WorldWideScience

Sample records for open shell nuclei

  1. Generalized seniority with realistic interactions in open-shell nuclei

    CERN Document Server

    Caprio, M A; Cai, K; Constantinou, Ch; Hellemans, V

    2014-01-01

    Generalized seniority provides a truncation scheme for the nuclear shell model, based on pairing correlations, which offers the possibility of dramatically reducing the dimensionality of the nuclear shell-model problem. Systematic comparisons against results obtained in the full shell-model space are required to assess the viability of this scheme. Here, we extend recent generalized seniority calculations for semimagic nuclei, the Ca isotopes, to open-shell nuclei, with both valence protons and valence neutrons. The even-mass Ti and Cr isotopes are treated in a full major shell and with realistic interactions, in the generalized seniority scheme with one broken proton pair and one broken neutron pair. Results for level energies, orbital occupations, and electromagnetic observables are compared with those obtained in the full shell-model space. We demonstrate that, even for the Ti isotopes, significant benefit would be obtained in going beyond the approximation of one broken pair of each type, while the Cr iso...

  2. In-medium similarity renormalization group for closed and open-shell nuclei

    Science.gov (United States)

    Hergert, H.

    2017-02-01

    We present a pedagogical introduction to the in-medium similarity renormalization group (IMSRG) framework for ab initio calculations of nuclei. The IMSRG performs continuous unitary transformations of the nuclear many-body Hamiltonian in second-quantized form, which can be implemented with polynomial computational effort. Through suitably chosen generators, it is possible to extract eigenvalues of the Hamiltonian in a given nucleus, or drive the Hamiltonian matrix in configuration space to specific structures, e.g., band- or block-diagonal form. Exploiting this flexibility, we describe two complementary approaches for the description of closed- and open-shell nuclei: the first is the multireference IMSRG (MR-IMSRG), which is designed for the efficient calculation of nuclear ground-state properties. The second is the derivation of non-empirical valence-space interactions that can be used as input for nuclear shell model (i.e., configuration interaction (CI)) calculations. This IMSRG+shell model approach provides immediate access to excitation spectra, transitions, etc, but is limited in applicability by the factorial cost of the CI calculations. We review applications of the MR-IMSRG and IMSRG+shell model approaches to the calculation of ground-state properties for the oxygen, calcium, and nickel isotopic chains or the spectroscopy of nuclei in the lower sd shell, respectively, and present selected new results, e.g., for the ground- and excited state properties of neon isotopes.

  3. Ab initio Bogoliubov coupled cluster theory for open-shell nuclei

    CERN Document Server

    Signoracci, Angelo; Hagen, Gaute; Jansen, Gustav

    2014-01-01

    Ab initio many-body methods address closed-shell nuclei up to mass A ~ 130 on the basis of realistic two- and three-nucleon interactions. Several routes to address open-shell nuclei are currently under investigation, including ideas which exploit spontaneous symmetry breaking. Singly open-shell nuclei can be efficiently described via the sole breaking of $U(1)$ gauge symmetry associated with particle number conservation, to account for their superfluid character. The present work formulates and applies Bogoliubov coupled cluster (BCC) theory, which consists of representing the exact ground-state wavefunction of the system as the exponential of a quasiparticle excitation cluster operator acting on a Bogoliubov reference state. Equations for the ground-state energy and cluster amplitudes are derived at the singles and doubles level (BCCSD) both algebraically and diagrammatically. The formalism includes three-nucleon forces at the normal-ordered two-body level. The first BCC code is implemented in $m$-scheme, wh...

  4. Ab initio Bogoliubov coupled cluster theory for open-shell nuclei

    Science.gov (United States)

    Signoracci, A.; Duguet, T.; Hagen, G.; Jansen, G. R.

    2015-06-01

    Background: Ab initio many-body methods have been developed over the past 10 yr to address closed-shell nuclei up to mass A ≈130 on the basis of realistic two- and three-nucleon interactions. A current frontier relates to the extension of those many-body methods to the description of open-shell nuclei. Several routes to address open-shell nuclei are currently under investigation, including ideas that exploit spontaneous symmetry breaking. Purpose: Singly open-shell nuclei can be efficiently described via the sole breaking of U(1) gauge symmetry associated with particle-number conservation as a way to account for their superfluid character. While this route was recently followed within the framework of self-consistent Green's function theory, the goal of the present work is to formulate a similar extension within the framework of coupled cluster theory. Methods: We formulate and apply Bogoliubov coupled cluster (BCC) theory, which consists of representing the exact ground-state wave function of the system as the exponential of a quasiparticle excitation cluster operator acting on a Bogoliubov reference state. Equations for the ground-state energy and the cluster amplitudes are derived at the singles and doubles level (BCCSD) both algebraically and diagrammatically. The formalism includes three-nucleon forces at the normal-ordered two-body level. The first BCC code is implemented in m scheme, which will permit the treatment of doubly open-shell nuclei via the further breaking of SU(2) symmetry associated with angular momentum conservation. Results: Proof-of-principle calculations in an Nmax=6 spherical harmonic oscillator basis for O,1816 and 18Ne in the BCCD approximation are in good agreement with standard coupled cluster results with the same chiral two-nucleon interaction, while 20O and 20Mg display underbinding relative to experiment. The breaking of U(1) symmetry, monitored by computing the variance associated with the particle-number operator, is relatively

  5. In-Medium Similarity Renormalization Group for Closed and Open-Shell Nuclei

    CERN Document Server

    Hergert, H

    2016-01-01

    We present a pedagogical introduction to the In-Medium Similarity Renormalization Group (IM-SRG) framework for ab initio calculations of nuclei. The IM-SRG performs continuous unitary transformations of the nuclear many-body Hamiltonian in second-quantized form, which can be implemented with polynomial computational effort. Through suitably chosen generators, it is possible to extract eigenvalues of the Hamiltonian in a given nucleus, or drive the Hamiltonian matrix in configuration space to specific structures, e.g., band- or block-diagonal form. Exploiting this flexibility, we describe two complementary approaches for the description of closed- and open-shell nuclei: The first is the Multireference IM-SRG (MR-IM-SRG), which is designed for the efficient calculation of nuclear ground-state properties. The second is the derivation of nonempirical valence-space interactions that can be used as input for nuclear Shell model (i.e., configuration interaction (CI)) calculations. This IM-SRG+Shell model approach pr...

  6. Ab Initio Description of Open-Shell Nuclei: Merging No-Core Shell Model and In-Medium Similarity Renormalization Group

    CERN Document Server

    Gebrerufael, Eskendr; Hergert, Heiko; Roth, Robert

    2016-01-01

    We merge two successful ab initio nuclear-structure methods, the no-core shell model (NCSM) and the multi-reference in-medium similarity renormalization group (IM-SRG) to define a new many-body approach for the comprehensive description of ground and excited states of closed and open-shell nuclei. Building on the key advantages of the two methods---the decoupling of excitations at the many-body level in the IM-SRG and the access to arbitrary nuclei, eigenstates, and observables in the NCSM---their combination enables fully converged no-core calculations for an unprecedented range of nuclei and observables at moderate computational cost. We present applications in the carbon and oxygen isotopic chains, where conventional NCSM calculations are still feasible and provide an important benchmark. The efficiency and rapid convergence of the new approach make it ideally suited for ab initio studies of the complete spectroscopy of nuclei up into the medium-mass regime.

  7. Ab Initio Description of Open-Shell Nuclei: Merging No-Core Shell Model and In-Medium Similarity Renormalization Group.

    Science.gov (United States)

    Gebrerufael, Eskendr; Vobig, Klaus; Hergert, Heiko; Roth, Robert

    2017-04-14

    We merge two successful ab initio nuclear-structure methods, the no-core shell model (NCSM) and the multireference in-medium similarity renormalization group (IM-SRG) to define a new many-body approach for the comprehensive description of ground and excited states of closed and open-shell nuclei. Building on the key advantages of the two methods-the decoupling of excitations at the many-body level in the IM-SRG and the access to arbitrary nuclei, eigenstates, and observables in the NCSM-their combination enables fully converged no-core calculations for an unprecedented range of nuclei and observables at moderate computational cost. We present applications in the carbon and oxygen isotopic chains, where conventional NCSM calculations are still feasible and provide an important benchmark. The efficiency and rapid convergence of the new approach make it ideally suited for ab initio studies of the complete spectroscopy of nuclei up into the medium-mass regime.

  8. Ground and excited states of doubly open-shell nuclei from ab initio valence-space Hamiltonians

    CERN Document Server

    Stroberg, S R; Holt, J D; Bogner, S K; Schwenk, A

    2015-01-01

    We present ab initio predictions for ground and excited states of doubly open-shell fluorine and neon isotopes based on chiral two- and three-nucleon interactions. We use the in-medium similarity renormalization group, in both flow-equation and Magnus formulations, to derive mass-dependent sd valence-space Hamiltonians. The experimental ground-state energies are reproduced through neutron number N=14, beyond which a new targeted normal-ordering procedure improves agreement with data and large-scale multi-reference calculations. For spectroscopy, we focus on neutron-rich 23-26F and 24-26Ne isotopes near N=14,16 magic numbers. In all cases we find an agreement with experiment competitive with established phenomenology. Moreover, yrast states are well described in 20Ne and 24Mg, providing an ab initio description of deformation in the medium-mass region.

  9. Shell structure of nuclei far from stability

    CERN Document Server

    Grawe, H

    2001-01-01

    The experimental status of shell structure studies in medium-heavy nuclei far off the line of beta-stability is reviewed. Experimental techniques, signatures for shell closure and expectations for future investigations are discussed for the key regions around sup 4 sup 8 sup , sup 5 sup 6 Ni, sup 1 sup 0 sup 0 Sn for proton rich nuclei and the neutron-rich N=20 isotones, Ca, Ni and Sn isotopes.

  10. Deformed $sd$-shell nuclei from first principles

    CERN Document Server

    Jansen, G R; Hagen, G; Navrátil, P

    2015-01-01

    We extend the ab initio coupled-cluster effective interaction (CCEI) method to deformed open-shell nuclei with protons and neutrons in the valence space, and compute binding energies and excited states of isotopes of neon and magnesium. We employ a nucleon-nucleon and three-nucleon interaction from chiral effective field theory evolved to a lower cutoff via a similarity renormalization group transformation. We find good agreement with experiment for binding energies and spectra, while charge radii of neon isotopes are underestimated. For the deformed nuclei $^{20}$Ne and $^{24}$Mg we reproduce rotational bands and electric quadrupole transitions within uncertainties estimated from an effective field theory for deformed nuclei, thereby demonstrating that collective phenomena in $sd$-shell nuclei emerge from complex ab initio calculations.

  11. Multi-Shell Shell Model for Heavy Nuclei

    OpenAIRE

    Sun, Yang; Wu, Cheng-Li

    2003-01-01

    Performing a shell model calculation for heavy nuclei has been a long-standing problem in nuclear physics. Here we propose one possible solution. The central idea of this proposal is to take the advantages of two existing models, the Projected Shell Model (PSM) and the Fermion Dynamical Symmetry Model (FDSM), to construct a multi-shell shell model. The PSM is an efficient method of coupling quasi-particle excitations to the high-spin rotational motion, whereas the FDSM contains a successful t...

  12. Multi-Shell Shell Model for Heavy Nuclei

    CERN Document Server

    Sun, Y; Sun, Yang; Wu, Cheng-Li

    2003-01-01

    Performing a shell model calculation for heavy nuclei has been a long-standing problem in nuclear physics. Here we propose one possible solution. The central idea of this proposal is to take the advantages of two existing models, the Projected Shell Model (PSM) and the Fermion Dynamical Symmetry Model (FDSM), to construct a multi-shell shell model. The PSM is an efficient method of coupling quasi-particle excitations to the high-spin rotational motion, whereas the FDSM contains a successful truncation scheme for the low-spin collective modes from the spherical to the well-deformed region. The new shell model is expected to describe simultaneously the single-particle and the low-lying collective excitations of all known types, yet keeping the model space tractable even for the heaviest nuclear systems.

  13. Shell model for warm rotating nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Matsuo, M.; Yoshida, K. [Kyoto Univ. (Japan); Dossing, T. [Univ. of Copenhagen (Denmark)] [and others

    1996-12-31

    Utilizing a shell model which combines the cranked Nilsson mean-field and the residual surface and volume delta two-body forces, the authors discuss the onset of rotational damping in normal- and super-deformed nuclei. Calculation for a typical normal deformed nucleus {sup 168}Yb indicates that the rotational damping sets in at around 0.8 MeV above the yrast line, and about 30 rotational bands of various length exists at a given rotational frequency, in overall agreement with experimental findings. It is predicted that the onset of rotational damping changes significantly in different superdeformed nuclei due to the variety of the shell gaps and single-particle orbits associated with the superdeformed mean-field.

  14. Shell Model for Warm Rotating Nuclei

    CERN Document Server

    Matsuo, M; Vigezzi, E; Broglia, R A; Yoshida, K

    1997-01-01

    In order to provide a microscopic description of levels and E2 transitions in rapidly rotating nuclei with internal excitation energy up to a few MeV, use is made of a shell model which combines the cranked Nilsson mean-field and the residual surface delta two-body force. The damping of collective rotational motion is investigated in the case of a typical rare-earth nucleus, namely \\Yb. It is found that rotational damping sets in at around 0.8 MeV above the yrast line, and the levels which form rotational band structures are thus limited. We predict at a given rotational frequency existence of about 30 rotational bands of various lengths, in overall agreement with the experimental findings. The onset of the rotational damping proceeds quite gradually as a function of the internal excitation energy. The transition region extends up to around 2 MeV above yrast and it is characterized by the presence of scars of discrete rotational bands which extend over few spin values and stand out among the damped transition...

  15. Shell correction energy for bubble nuclei

    CERN Document Server

    Yu, Y; Magierski, P; Bulgac, Aurel; Magierski, Piotr

    2000-01-01

    The positioning of a bubble inside a many fermion system does not affect the volume, surface or curvature terms in the liquid drop expansion of the total energy. Besides possible Coulomb effects, the only other contribution to the ground state energy of such a system arises from shell effects. We show that the potential energy surface is a rather shallow function of the displacement of the bubble from the center and in most cases the preferential position of a bubble is off center. Systems with bubbles are expected to have bands of extremely low lying collective states, corresponding to various bubble displacements.

  16. Three-nucleon forces in exotic open-shell isotopes

    CERN Document Server

    Soma, V; Cipollone, A; Duguet, T; Navratil, P

    2013-01-01

    Advances in the self-consistent Green's function approach to finite nuclei are discussed, including the implementation of three-nucleon forces and the extension to the Gorkov formalism. We report results on binding energies in the nitrogen and fluorine isotopic chains, as well as spectral functions of 22O. The application to medium-mass open-shell systems is illustrated by separation energy spectra of two argon isotopes, which are compared to one-neutron removal experiments.

  17. Mean-field approach to collective excitations in deformed sd-shell nuclei using realistic interactions

    Energy Technology Data Exchange (ETDEWEB)

    Erler, Bastian

    2012-07-18

    Realistic nucleon-nucleon interactions transformed via the Unitary Correlation Operator Method (UCOM) or the Similarity Renormalization Group (SRG) have proven to be a suitable starting point for the description of closed-shell nuclei via mean-field methods like Hartree-Fock (HF). This allows the treatment of a number of heavy nuclei with realistic nucleon-nucleon interactions, which would otherwise only be possible with phenomenological interactions. To include three-nucleon forces in an approximate way, the UCOM or SRG transformed interactions can be augmented by a three-body contact interaction, which is necessary to reproduce measured charge radii. However, many interesting nuclei, including those near the neutron drip line, are far away from closed shells. These nuclei are of great importance for modeling nucleosynthesis processes in the universe, but experiments can only be performed at a few research facilities. In this work, the Hartree Fock (HF) approach with realistic interactions is extended to light deformed nuclei. Pairing correlations are not taken into account. A crucial step in this process is to allow deformed ground states on the mean-field level, as only nuclei with at least one closed shell can be described with spherical HF ground states. To restore the rotational symmetry in the lab frame, exact angular-momentum projection (AMP) is implemented. Constrained HF calculations are used for an approximate variation after projection approach. The AMP-HF description of open-shell nuclei is on par with the pure HF description of closed-shell nuclei. Charge-radii and systematics of binding energies agree well with experiment. However, missing correlations, lead to an underestimated absolute value of the binding energy. Projection on higher angular momenta approximately reproduces the energy systematics of rotational bands. To describe collective excitations, the Random Phase Approximation (RPA) constitutes a well tested approach, which can also be

  18. Shell-model calculations of nuclei around mass 130

    Science.gov (United States)

    Teruya, E.; Yoshinaga, N.; Higashiyama, K.; Odahara, A.

    2015-09-01

    Shell-model calculations are performed for even-even, odd-mass, and doubly-odd nuclei of Sn, Sb, Te, I, Xe, Cs, and Ba isotopes around mass 130 using the single-particle space made up of valence nucleons occupying the 0 g7 /2 ,1 d5 /2 ,2 s1 /2 ,0 h11 /2 , and 1 d3 /2 orbitals. The calculated energies and electromagnetic transitions are compared with the experimental data. In addition, several typical isomers in this region are investigated.

  19. Unified description of pf-shell nuclei by the Monte Carlo shell model calculations

    Energy Technology Data Exchange (ETDEWEB)

    Mizusaki, Takahiro; Otsuka, Takaharu [Tokyo Univ. (Japan). Dept. of Physics; Honma, Michio

    1998-03-01

    The attempts to solve shell model by new methods are briefed. The shell model calculation by quantum Monte Carlo diagonalization which was proposed by the authors is a more practical method, and it became to be known that it can solve the problem with sufficiently good accuracy. As to the treatment of angular momentum, in the method of the authors, deformed Slater determinant is used as the basis, therefore, for making angular momentum into the peculiar state, projected operator is used. The space determined dynamically is treated mainly stochastically, and the energy of the multibody by the basis formed as the result is evaluated and selectively adopted. The symmetry is discussed, and the method of decomposing shell model space into dynamically determined space and the product of spin and isospin spaces was devised. The calculation processes are shown with the example of {sup 50}Mn nuclei. The calculation of the level structure of {sup 48}Cr with known exact energy can be done with the accuracy of peculiar absolute energy value within 200 keV. {sup 56}Ni nuclei are the self-conjugate nuclei of Z=N=28. The results of the shell model calculation of {sup 56}Ni nucleus structure by using the interactions of nuclear models are reported. (K.I.)

  20. Unified description of pf-shell nuclei by the Monte Carlo shell model calculations

    Energy Technology Data Exchange (ETDEWEB)

    Mizusaki, Takahiro; Otsuka, Takaharu [Tokyo Univ. (Japan). Dept. of Physics; Honma, Michio

    1998-03-01

    The attempts to solve shell model by new methods are briefed. The shell model calculation by quantum Monte Carlo diagonalization which was proposed by the authors is a more practical method, and it became to be known that it can solve the problem with sufficiently good accuracy. As to the treatment of angular momentum, in the method of the authors, deformed Slater determinant is used as the basis, therefore, for making angular momentum into the peculiar state, projected operator is used. The space determined dynamically is treated mainly stochastically, and the energy of the multibody by the basis formed as the result is evaluated and selectively adopted. The symmetry is discussed, and the method of decomposing shell model space into dynamically determined space and the product of spin and isospin spaces was devised. The calculation processes are shown with the example of {sup 50}Mn nuclei. The calculation of the level structure of {sup 48}Cr with known exact energy can be done with the accuracy of peculiar absolute energy value within 200 keV. {sup 56}Ni nuclei are the self-conjugate nuclei of Z=N=28. The results of the shell model calculation of {sup 56}Ni nucleus structure by using the interactions of nuclear models are reported. (K.I.)

  1. Shell-model studies of the N=14 and 16 shell closures in neutron-rich nuclei

    Institute of Scientific and Technical Information of China (English)

    YUAN Cen-Xi; QI Chong; XU Fu-Rong

    2009-01-01

    Shell-model studies on the N = 14 and 16 shell closures in neutron-rich Be, C, O and Ne isotopes are presented. We calculate, with the WBT interaction, the excited states in these nuclei. The calculations agree with recent experiment data. Excited energies and B(E2) values are displayed to discuss the shell closures.Our results support the N = 16 shell closure in these isotopes, while indicating a disappearance of N = 14 shell closure in Be and C isotopes.

  2. Benchmark calculation of no-core Monte Carlo shell model in light nuclei

    CERN Document Server

    Abe, T; Otsuka, T; Shimizu, N; Utsuno, Y; Vary, J P; 10.1063/1.3584062

    2011-01-01

    The Monte Carlo shell model is firstly applied to the calculation of the no-core shell model in light nuclei. The results are compared with those of the full configuration interaction. The agreements between them are within a few % at most.

  3. First-principles results for electromagnetic properties of s d shell nuclei

    Science.gov (United States)

    Saxena, Archana; Srivastava, Praveen C.

    2017-08-01

    In this work we present ab initio shell-model calculations for electric quadrupole moments and magnetic dipole moments of s d shell nuclei using valence-space Hamiltonians derived with two ab initio approaches: the in-medium similarity renormalization group (IM-SRG) and the coupled-cluster effective interaction (CCEI). Results are in reasonable agreement with the available experimental data as well as with the results from the phenomenological USDB effective interaction. This work will add more information to the available ab initio results for the spectroscopy of s d shell nuclei.

  4. The shell model—simplicity from complexity: some of my best nuclei are spherical

    Science.gov (United States)

    Talmi, Igal

    2017-08-01

    This article presents shell model applications to spherical nuclei with strong emphasis on semi-magic ones. A successful description of their low lying levels is obtained by applying to them the spherical shell model. These spherical nuclei are rather different from nuclei which exhibit collective phenomena, like rotational spectra. In the present article, several applications of the shell model to nuclei are presented. Only simple cases are considered which do not involve complicated calculations. These cases are sufficient to demonstrate the power of the shell model and to find the important ingredients of the mutual interactions of nucleons. The latter are limited to two-body interactions and it seems that they are the important ones in determination of the structure of nuclei. The interaction which should be used in the shell model (effective interaction) is a highly renormalized version of the bare interaction, between free nucleons. In the absence of a reliable many-body theory of the nucleus, matrix elements of the effective interaction are determined from energies of actual nuclei. General features of these are discussed, with particular attention to matrix elements which lead to nuclear deformation and rotational spectra.

  5. Shell Effect of Superheavy Nuclei in Self-consistent Mean-Field Models

    Institute of Scientific and Technical Information of China (English)

    RENZhong-Zhou; TAIFei; XUChang; CHENDing-Han; ZHANGHu-Yong; CAIXiang-Zhou; SHENWen-Qing

    2004-01-01

    We analyze in detail the numerical results of superheavy nuclei in deformed relativistic mean-field model and deformed Skyrme-Hartree-Fock model. The common points and differences of both models are systematically compared and discussed. Their consequences on the stability of superheavy nuclei are explored and explained. The theoreticalresults are compared with new data of superheavy nuclei from GSI and from Dubna and reasonable agreement is reached.Nuclear shell effect in superheavy region is analyzed and discussed. The spherical shell effect disappears in some cases due to the appearance of deformation or superdeformation in the ground states of nuclei, where valence nucleons occupysignificantly the intruder levels of nuclei. It is shown for the first time that the significant occupation of vaJence nucleons on the intruder states plays an important role for the ground state properties of superheavy nuclei. Nuclei are stable in the deformed or superdeformed configurations. We further point out that one cannot obtain the octupole deformation of even-even nuclei in the present relativistic mean-field model with the σ,ω and ρ mesons because there is no parityviolating interaction and the conservation of parity of even-even nuclei is a basic assumption of the present relativistic mean-field model.

  6. Gross shell structure at high spin in heavy nuclei

    CERN Document Server

    Deleplanque, M A; Pashkevich, V V; Chu, S Y; Unzhakova, A

    2004-01-01

    Experimental nuclear moments of inertia at high spins along the yrast line have been determined systematically and found to differ from the rigid-body values. The difference is attributed to shell effects and these have been calculated microscopically. The data and quantal calculations are interpreted by means of the semiclassical Periodic Orbit Theory. From this new perspective, features in the moments of inertia as a function of neutron number and spin, as well as their relation to the shell energies can be understood. Gross shell effects persist up to the highest angular momenta observed.

  7. Gross shell structure at high spin in heavy nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Deleplanque, Marie-Agnes; Frauendorf, Stefan; Pashkevich, Vitaly V.; Chu, S.Y.; Unzhakova, Anja

    2003-10-07

    Experimental nuclear moments of inertia at high spins along the yrast line have been determined systematically and found to differ from the rigid-body values. The difference is attributed to shell effect and these have been calculated microscopically. The data and quantal calculations are interpreted by means of the semiclassical Periodic Orbit Theory. From this new perspective, features in the moments of inertia as a function of neutron number and spin, as well as their relation to the shell energies can be understood. Gross shell effects persist up to the highest angular momenta observed.

  8. Coupled cluster calculation for ground state properties of closed-shell nuclei and single hole states.

    Science.gov (United States)

    Mihaila, Bogdan; Heisenberg, Jochen

    2000-04-01

    We continue the investigations of ground state properties of closed-shell nuclei using the Argonne v18 realistic NN potential, together with the Urbana IX three-nucleon interaction. The ground state wave function is used to calculate the charge form factor and charge density. Starting with the ground state wave function of the closed-shell nucleus, we use the equation of motion technique to calculate the ground state and excited states of a neighboring nucleus. We then generate the corresponding magnetic form factor. We correct for distortions due to the interaction between the electron probe and the nuclear Coulomb field using the DWBA picture. We compare our results with the available experimental data. Even though our presentation will focus mainly on the ^16O and ^15N nuclei, results for other nuclei in the p and s-d shell will also be presented.

  9. Constrained Hartree-Fock Theory and Study of Deformed Structures of Closed Shell Nuclei

    Science.gov (United States)

    Praharaj, Choudhury

    2016-03-01

    We have studied some N or Z = 50 nuclei in a microscopic model with effective interaction in a reasonably large shell model space. Excitation of particles across 50 shell closure leads to well-deformed excited prolate configurations. The potential energy surfaces of nuclei are studied using Hartree-Fock theory with quadrupole constraint to explore the various deformed configurations of N = 50 nuclei 82Ge , 84Se and 86Kr . Energy spectra are calculated from various intrinsic states using Peierls-Yoccoz angular momentum projection technique. Results of spectra and electromagnetic moments and transitions will be presented for N = 50 nuclei and for Z = 50 114Sn nucleus. Supported by Grant No SB/S2/HEP-06/2013 of DST.

  10. Ground state of medium-heavy doubly-closed shell nuclei in correlated basis function theory

    CERN Document Server

    Bisconti, C; Có, G; Fabrocini, A

    2006-01-01

    The correlated basis function theory is applied to the study of medium-heavy doubly closed shell nuclei with different wave functions for protons and neutrons and in the jj coupling scheme. State dependent correlations including tensor correlations are used. Realistic two-body interactions of Argonne and Urbana type, together with three-body interactions have been used to calculate ground state energies and density distributions of the 12C, 16O, 40Ca, 48Ca and 208Pb nuclei.

  11. Shell model for heavy nuclei and its application in nuclear astrophysics

    CERN Document Server

    Sun, Y

    2006-01-01

    Performing shell model calculations for heavy nuclei is a long-standing problem in nuclear physics. The shell model truncation in the configuration space is an unavoidable step. The Projected Shell Model (PSM) truncates the space under the guidance of the deformed mean-field solutions. This implies that the PSM uses a novel and efficient way to bridge the two conventional methods: the deformed mean-field approximations, which are widely applied to heavy nuclei but able to describe the physics only in the intrinsic frame, and the spherical shell model diagonalization method, which is most fundamental but feasible only for small systems. We discuss the basic philosophy in construction of the PSM (or generally PSM-like) approach. Several examples from the PSM calculations are presented. Astrophysical applications are emphasized.

  12. Systematization of α-decaying nuclei based on shell structures: The case of even-odd nuclei

    Science.gov (United States)

    Yarman, Tolga; Zaim, Nimet; Yarman, O.; Kholmetskii, Alexander; Arık, Metin

    2017-01-01

    Previously, we provided a novel systematization of α-decaying even-even nuclei starting with the classically adopted mechanism (Yarman et al., Eur. Phys. J. A 52, 140 (2016)). The decay half-life of an α-decaying nucleus was framed so that i) the α-particle is taken at the outset to be born inside the parent nucleus with a given probability, ii) where it then keeps on bouncing off of the barrier of the parent nucleus till iii) it finally tunnels through the barrier. Knowing beforehand the measured decay half-life, we have taken into consideration, as a parameter, the probability of the α-particle being first born within the parent before it is emitted. We thence developed a scaffold based on shell properties of families composed of alike even-even nuclei. Nevertheless, our model allows us to incorporate any α-decaying nuclei, and along this line, we present a follow-up systematization of even-odd nuclei, with cases of odd-even and odd-odd α-decaying nuclei pending to be considered in a separate contribution. Notwithstanding, we make an effort herein to expand our approach to investigate the effect of "pairing" ( e.g., when a number of nucleons in the given nucleus becomes an even number, instead of the initial odd number, due to the addition of at least one neutron). Our results show that "pairing", as expected, definitely increases the stability of the given nucleus.

  13. Statistical Spectroscopy for Neutron-rich sd-Shell Nuclei

    CERN Document Server

    Kar, Kamales

    2012-01-01

    Statistical spectroscopic results using the spectral distribution theory are obtained for the structure of neutron-rich light nuclei going towards the drip line and compared to experimental values available. These results will be useful for nuclear astrophysics problems where often averaged nuclear properties are adequate.

  14. Evolution of Structure in Nuclei: Meditation by Sub-Shell Modifications and Relation to Binding Energies

    Science.gov (United States)

    Casten, R. F.; Cakirli, R. B.

    2009-03-01

    Understanding the development of configuration mixing, coherence, collectivity, and deformation in nuclei is one of the crucial challenges in nuclear structure physics, and one which has become all the more important with the advent of next generation facilities for the study of exotic nuclei. We will discuss recent work on phase/shape transitional behavior in nuclei, and the role of changes in sub-shell structure in mediating such transitional regions. We will also discuss a newly found, much deeper, link between nuclear structure and nuclear binding energies.

  15. Semiclassical Calculation of Shell Effects in Deformed Nuclei

    CERN Document Server

    Brack, M

    2000-01-01

    We summarize recent work in which the shell effect, which causes the onset of the mass asymmetry in nuclear fission, could be explained semiclassically in the framework of the periodic orbit theory. We also present new results for the inclusion of a spin-orbit interaction in the semiclassical calculation of the level density.

  16. Parity violation in quasielastic electron scattering from closed-shell nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Amaro, J.E. [Massachusetts Inst. of Technol., Cambridge, MA (United States). Dept. of Phys.]|[Departamento de Fisica Moderna, Universidad de Granada, E-18071 Granada (Spain); Caballero, J.A. [Instituto de Estructura de la Materia, Consejo Superior de Investigaciones Cientificas, Serrano 123, Madrid 28006 (Spain); Donnelly, T.W. [Massachusetts Inst. of Technol., Cambridge, MA (United States). Dept. of Phys.; Lallena, A.M. [Departamento de Fisica Moderna, Universidad de Granada, E-18071 Granada (Spain); Moya de Guerra, E. [Instituto de Estructura de la Materia, Consejo Superior de Investigaciones Cientificas, Serrano 123, Madrid 28006 (Spain); Udias, J.M. [National Laboratory for Nuclear and High-Energy Physics, Section K (NIKHEF-K), P.O. Box 41882, NL-1009 DB Amsterdam (Netherlands)

    1996-06-03

    The electromagnetic and weak neutral current matrix elements that enter in the analysis of parity-violating quasielastic electron scattering are calculated using a continuum nuclear shell model. New approximations to the on-shell relativistic one-body currents and relativistic kinematics for use in such models are developed and discussed in detail. Results are presented for three closed-shell nuclei of interest: {sup 16}O, {sup 40}Ca and {sup 208}Pb. The current work concludes with a study of the sensitivity of the resulting parity-violating asymmetries to properties of the nucleon form factors including the possible strangeness content of the nucleon. (orig.).

  17. Inclusion of temperature dependent shell corrections in Landau theory for hot rotating nuclei

    Indian Academy of Sciences (India)

    G Shanmugam; P Arumugam

    2001-07-01

    Landau theory used for studying hot rotating nuclei usually uses zero temperature Strutinsky smoothed total energy for the temperature dependent shell corrections. This is replaced in this work by the temperature dependent Strutinsky smoothed free energy. Our results show that this replacement has only marginal effect for temperatures greater than 1 MeV but plays significant role at lower temperatures.

  18. Probing Shell Correction at High Spin by Neutron Emission of Doubly Magic Nuclei 208pb and 132Sn

    Institute of Scientific and Technical Information of China (English)

    YEWei

    2005-01-01

    Shell effects in particle emission for two doubly magic nuclei 132Sn and 208pb were studied in the framework of Smoluchowski equation taking into account temperature and spin-dependent shell correction. It is shown that the shelle ffects in the emission of pre-scission neutrons are sensitive to the spin dependence of the shell correction at a moderate excitation energy. Therefore, we propose to use neutron multiplicity as an observable to probe the shell correction at high spins.

  19. Probing Shell Correction at High Spin by Neutron Emission of Doubly Magic Nuclei 208pb and 132Sn

    Institute of Scientific and Technical Information of China (English)

    YE Wei

    2005-01-01

    Shell effects in particle emission for two doubly magic nuclei 132 Sn and 208 Pb were studied in the framework of Smoluchowski equation taking into account temperature and spin-dependent shell correction. It is shown that the shell effects in the enission of pre-scission neutrons are sensitive to the spin dependence of the shell correction at a moderate excitation energy. Therefore, we propose to use neutron multiplicity as an observable to probe the shell correction at high spins.

  20. Isospin Symmetry Violation in sd-Shell Nuclei

    Directory of Open Access Journals (Sweden)

    Lam Yi Hua

    2014-03-01

    Full Text Available We construct a new set of isospin-nonconserving (INC shell-model Hamiltonians and apply it (i to study the isobaric-mass multiplet equation (IMME beyond a quadratic form in the A = 35, 3/2+ quartet, (ii to compute the isospin mixing corrections to superallowed Fermi branch of 1+ → 1+ β decay of 32Cl, and (iii to obtain the isospin-forbidden branching ratios of β-delayed proton emission from 25Si.

  1. Collectivity in Heavy Nuclei in the Shell Model Monte Carlo Approach

    CERN Document Server

    Özen, C; Nakada, H

    2013-01-01

    The microscopic description of collectivity in heavy nuclei in the framework of the configuration-interaction shell model has been a major challenge. The size of the model space required for the description of heavy nuclei prohibits the use of conventional diagonalization methods. We have overcome this difficulty by using the shell model Monte Carlo (SMMC) method, which can treat model spaces that are many orders of magnitude larger than those that can be treated by conventional methods. We identify a thermal observable that can distinguish between vibrational and rotational collectivity and use it to describe the crossover from vibrational to rotational collectivity in families of even-even rare-earth isotopes. We calculate the state densities in these nuclei and find them to be in close agreement with experimental data. We also calculate the collective enhancement factors of the corresponding level densities and find that their decay with excitation energy is correlated with the pairing and shape phase tran...

  2. Nuclear β --decay half-lives for {fp} and {fpg} shell nuclei

    Science.gov (United States)

    Kumar, Vikas; Srivastava, P. C.; Li, Hantao

    2016-10-01

    In the present work we calculate the allowed {β }--decay half-lives of nuclei with Z=20-30 and N ≤slant 50 systematically under the framework of the nuclear shell model. A recent study shows that some nuclei in this region belong to the island of inversion. We perform calculation for fp shell nuclei using the KB3G effective interaction. In the case of Ni, Cu, and Zn, we used the JUN45 effective interaction. Theoretical results of Q values, half-lives, excitation energies, logft values, and branching fractions are discussed and compared with the experimental data. In the Ni region, we also compared our calculated results with recent experimental data (Xu et al 2014 Phys. Rev. Lett. 113 032505). The present results agree with the experimental data of half-lives in comparison to QRPA.

  3. Shell model approach for nuclei with mass around 220

    Science.gov (United States)

    Kaiura, Yukiko; Yoshinaga, Naotaka; Higashiyama, Koji

    2014-09-01

    Ra and Th isotopes with mass around 220 belonging to a transitional region between spherical and deformed regions have fascinated our interest from the past. In particular, since a large number of negative parity states are observed in low-lying states, collective octupole correlations are supposed to be important. In this talk we report the nuclear structure of Po, Rn, Ra and Th isotopes in terms of the pair truncated shell model, the basic ingredients of which consist of nuclear collective models. The 208Pb is considered as the doubly-magic core. The conventional pairing plus quadrupole interaction is employed. Energy levels and electric transitions are compared between theory and experiment.

  4. Statistical theory of light nucleus reactions with 1p-shell light nuclei

    Science.gov (United States)

    Xiaojun, Sun; Jingshang, Zhang

    2017-09-01

    The 1p-shell light elements (Li, Be, B, C, N, and O) had long been selected as the most important materials for improving neutron economy in thermal and fast fission reactors and in the design of accelerator-driven spallation neutron sources. A statistical theory of light nucleus reactions (STLN) is proposed to describe the double-differential cross sections for both neutron and light charged particle induced nuclear reactions with 1p-shell light nuclei. The dynamics of STLN is described by the unified Hauser-Feshbach and exciton model, in which the angular momentum and parity conservations are strictly considered in equilibrium and pre-equilibrium processes. The Coulomb barriers of the incoming and outgoing charged particles, which significantly influence the open channels of the reaction, can be reasonably considered in incident channel and different outgoing channels. In kinematics, the recoiling effects in various emission processes are strictly taken into account. The analytical energy and angular spectra of the reaction products in sequential and simultaneous emission processes are obtained in terms of the new integral formula proposed in our recent paper. Taking 12C(n, xn), 9Be(n, xn), 16O(n, xn), and 9Be(p,xn) reactions as examples, we had calculated the double-differential cross sections of outgoing neutrons and compared with the experimental data. In addition, we had also calculated the partition and total kerma coefficients for 12C(n, xn) and 16O(n, xn) reactions, respectively. The existing experimental data can be remarkably well reproduced by STLN, which had been used to set up file-6 in CENDL database.

  5. Collective excitations in deformed sd-shell nuclei from realistic interactions

    CERN Document Server

    Erler, Bastian

    2014-01-01

    Background: Collective excitations of nuclei and their theoretical descriptions provide an insight into the structure of nuclei. Replacing traditional phenomenological interactions with unitarily transformed realistic nucleon-nucleon interactions increases the predictive power of the theoretical calculations for exotic or deformed nuclei. Purpose: Extend the application of realistic interactions to deformed nuclei and compare the performance of different interactions, including phenomenological interactions, for collective excitations in the sd-shell. Method: Ground-state energies and charge radii of 20-Ne, 28-Si and 32-S are calculated with the Hartree-Fock method. Transition strengths and transition densities are obtained in the Random Phase Approximation with explicit angular-momentum projection. Results: Strength distributions for monopole, dipole and quadrupole excitations are analyzed and compared to experimental data. Transition densities give insight into the structure of collective excitations in def...

  6. A novel approach to the systematization of α-decaying nuclei, based on shell structures

    Science.gov (United States)

    Yarman, Tolga; Zaim, Nimet; Amon Susam, Lidya; Kholmetskii, Alexander; Arık, Metin; Azmi Altıntaş, Ali; Ozaydin, Fatih

    2016-05-01

    We provide a novel systematization of α-decaying nuclei, starting with the classically adopted mechanism. The decay half-life of an α-disintegrating nucleus is framed, supposing that i) the α-particle is born inside the parent, then ii) it keeps on hitting the barrier, while it runs back and forth inside the parent, and hitting each time the barrier, and iii) it finally tunnels through the barrier. One can, knowing the decay half-life, consider the probability that the α-particle is born within the parent, before it is emitted, as a parameter. Under all circumstances, the decay appears to be governed by the shell structure of the given nucleus. Our approach well allows to incorporate (not only even-even nuclei, but) all nuclei, decaying via throwing an alpha particle. Though herein, we limit ourselves with just even-even nuclei, in the aim of comparing our results with the existing Geiger-Nuttal results.

  7. Systematization of α-decaying nuclei based on shell structures: The case of even-odd nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Yarman, Tolga [Okan University, Istanbul (Turkey); Zaim, Nimet [Trakya University, Edirne (Turkey); Yarman, O. [Istanbul University, Istanbul (Turkey); Kholmetskii, Alexander [Belarusian State University, Minsk (Belarus); Arik, Metin [Bogazici University, Istanbul (Turkey)

    2017-01-15

    Previously, we provided a novel systematization of α-decaying even-even nuclei starting with the classically adopted mechanism (Yarman et al., Eur. Phys. J. A 52, 140 (2016)). The decay half-life of an α-decaying nucleus was framed so that i) the α-particle is taken at the outset to be born inside the parent nucleus with a given probability, ii) where it then keeps on bouncing off of the barrier of the parent nucleus till iii) it finally tunnels through the barrier. Knowing beforehand the measured decay half-life, we have taken into consideration, as a parameter, the probability of the α-particle being first born within the parent before it is emitted. We thence developed a scaffold based on shell properties of families composed of alike even-even nuclei. Nevertheless, our model allows us to incorporate any α-decaying nuclei, and along this line, we present a follow-up systematization of even-odd nuclei, with cases of odd-even and odd-odd α-decaying nuclei pending to be considered in a separate contribution. Notwithstanding, we make an effort herein to expand our approach to investigate the effect of ''pairing'' (e.g., when a number of nucleons in the given nucleus becomes an even number, instead of the initial odd number, due to the addition of at least one neutron). Our results show that ''pairing'', as expected, definitely increases the stability of the given nucleus. (orig.)

  8. Nuclear shell effect and collinear tripartition of nuclei

    CERN Document Server

    Nasirov, A K; Tashkhodjaev, R B

    2014-01-01

    A possibility of formation of the three reaction products having comparable masses at the spontaneous fission of $^{252}$Cf is theoretically explored. This work is aimed to study the mechanism leading to observation of the reaction products with masses $M_1=$136---140 and $M_2=$68---72 in coincidence by the FOBOS group in JINR. The same type of ternary fission decay has been observed in the reaction $^{235}$U(n$_{\\rm th}$,fff). The potential energy surface for the ternary system forming a collinear nuclear chain is calculated for the wide range of mass and charge numbers of constituent nuclei. The results of the PES for the tripartition of $^{252}$Cf(sf,fff) shows, that we have favorable dynamical conditions for the formation of fragments with mass combinations of clusters $^{68-70}$Ni with $^{130-132}$Sn and with missing cluster $^{48-52}$Ca.

  9. Nuclear shell effect and collinear tripartition of nuclei

    Indian Academy of Sciences (India)

    Avazbek K Nasirov; Wolfram von Oertzen; Rustam B Tashkhodjaev

    2015-08-01

    A possibility for the formation of three reaction products having comparable masses at the spontaneous fission of 252Cf is theoretically explored. This work is aimed to study the mechanism leading to the observation of the reaction products with masses $M_{1}$ = 136–140 and $M_{2}$ = 68–72 in coincidence with the FOBOS group in JINR. The same type of ternary fission decay has been observed in the 235U(nth, fff) reaction. The potential energy surface (PES) for the ternary system forming a collinear nuclear chain is calculated for a wide range of masses and charge numbers of the constituent nuclei. The results of the PES for the tripartition of 252Cf(sf, fff) allows us to establish dynamical conditions leading to the formation of fragments with mass combinations of clusters 68−70Ni with 130−132Sn and with the missing cluster 48−52Ca.

  10. Studies of short-lived nuclei in the proximity of closed shells

    Energy Technology Data Exchange (ETDEWEB)

    Omtvedt, J.P.

    1995-12-31

    In this work the structure of {sup 84,85}Se at the closed N=50 neutron shell, and the {sup 132}Sb, {sup 132}Sn, and {sup 134}Te nuclei, at the doubly closed N=82,Z=50 shells, was studied. The experiments were performed at the OSIRIS fission product mass separator at Studsvik, Sweden. The excited levels of the studied nuclei were populated in {beta} decay. The sources were produced in fission of {sup 235}U in the OSIRIS combined target and ion source. The nuclei were studied by standard nuclear spectroscopy measuring techniques: Singles {gamma} spectra and {gamma}{gamma}-coincidence data were obtained. In addition {gamma}{gamma}({theta}) angular correlation and {beta}{gamma}{gamma}(t) triple coincidence ``fast-timing`` ,measurements were performed on the nuclei in the {sup 132}Sn (N=82,Z=50) region. Detailed level schemes for the {sup 84,85}Se, {sup 132}Sb,{sup 132}Sn, {sup 132}Te nuclei were built, greatly improvi our knowledge of the structure of these nuclei. The experimentally deduced transition rates and multipole mixing ratios of the studied {sup 132}Sn region nuclei were compared to theoretical calculations within the random phase approximation framework and related models. Particular attention was paid to the collective properties of nuclei in the {sup 132}Sn region, parametrized by the electrical octupole effective charge. A range of general software spectroscopic tools were developed for the purpose of analysing the experimental data. This included a program, Yggdrasil, which for the first time allowed a complete two-dimensional {gamma}{gamma}-coincidence matrix to be analysed on ordinary ``small`` personal computers (PCs). 49 refs., 10 figs., 2 tabs.

  11. Nucleon momentum distributions and elastic electron scattering form factors for some 1p-shell nuclei

    Indian Academy of Sciences (India)

    A K Hamoudi; M A Hasan; A R Ridha

    2012-05-01

    The nucleon momentum distributions (NMD) and elastic electron scattering form factors of the ground state for 1p-shell nuclei with = (such as 6Li, 10B, 12C and 14N nuclei) have been calculated in the framework of the coherent density fluctuation model (CDFM) and expressed in terms of the weight function $|f(x)|^2$. The weight function has been expressed in terms of nucleon density distribution (NDD) of the nuclei and determined from the theory and the experiment. The feature of the long-tail behaviour at high-momentum region of the NMDs has been obtained by both the theoretical and experimental weight functions. The experimental form factors $F(q)$ of all the considered nuclei are very well reproduced by the present calculations for all values of momentum transfer . It is found that the contributions of the quadrupole form factors $F_{C2}(q)$ in 10B and 14N nuclei, which are described by the undeformed p-shell model, are essential for obtaining a remarkable agreement between the theoretical and experimental form factors.

  12. Exploring the changing of shell structure of nuclei at N=50

    Energy Technology Data Exchange (ETDEWEB)

    De Angelis, G. [Istituto Nazionale di Fisica Nucleare laboratori Nazionali di Legnaro, Legnaro (Italy); Duchene, G.; Faul, T. [IPHC, IN2P3/CNRS et Universite' Louis Pasteur, Strasbourg, (France)] (and others)

    2005-07-01

    Here it is reported an experimental study of the excited structures of the neutron-rich N=50 and 51 isotones. New experimental information has been obtained on a wide range of nuclei close to the N=50 shell closure by means of multi-nucleon transfer and deep-inelastic collisions. The reaction mechanism allows the population of medium and high-spin yrast states. The systematic of the N=51 single-neutron states, extended down to the Z=34, can be used to test the predictions of the shell evolution based on the effects of the tensor interactions as well as of the different effective interactions.

  13. No-Core Shell Model Calculations in Light Nuclei with Three-Nucleon Forces

    Energy Technology Data Exchange (ETDEWEB)

    Barrett, B R; Vary, J P; Nogga, A; Navratil, P; Ormand, W E

    2004-01-08

    The ab initio No-Core Shell Model (NCSM) has recently been expanded to include nucleon-nucleon (NN) and three-nucleon (3N) interactions at the three-body cluster level. Here it is used to predict binding energies and spectra of p-shell nuclei based on realistic NN and 3N interactions. It is shown that 3N force (3NF) properties can be studied in these nuclear systems. First results show that interactions based on chiral perturbation theory lead to a realistic description of {sup 6}Li.

  14. Large-scale shell-model calculations of nuclei around mass 210

    Science.gov (United States)

    Teruya, E.; Higashiyama, K.; Yoshinaga, N.

    2016-06-01

    Large-scale shell-model calculations are performed for even-even, odd-mass, and doubly odd nuclei of Pb, Bi, Po, At, Rn, and Fr isotopes in the neutron deficit region (Z ≥82 ,N ≤126 ) assuming 208Pb as a doubly magic core. All the six single-particle orbitals between the magic numbers 82 and 126, namely, 0 h9 /2,1 f7 /2,0 i13 /2,2 p3 /2,1 f5 /2 , and 2 p1 /2 , are considered. For a phenomenological effective two-body interaction, one set of the monopole pairing and quadrupole-quadrupole interactions including the multipole-pairing interactions is adopted for all the nuclei considered. The calculated energies and electromagnetic properties are compared with the experimental data. Furthermore, many isomeric states are analyzed in terms of the shell-model configurations.

  15. Triaxial projected shell model study of chiral rotation in odd-odd nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Bhat, G.H. [Department of Physics, University of Kashmir, Srinagar, 190 006 (India); Sheikh, J.A. [Department of Physics, University of Kashmir, Srinagar, 190 006 (India); Department of Physics and Astronomy, University of Tennessee, Knoxville, TN 37996 (United States); Palit, R., E-mail: palit@tifr.res.in [Department of Nuclear and Atomic Physics, Tata Institute of Fundamental Research, Colaba, Mumbai, 400 005 (India)

    2012-01-20

    Chiral rotation observed in {sup 128}Cs is studied using the newly developed microscopic triaxial projected shell model (TPSM) approach. The observed energy levels and the electromagnetic transition probabilities of the nearly degenerate chiral dipole bands in this isotope are well reproduced by the present model. This demonstrates the broad applicability of the TPSM approach, based on a schematic interaction and angular-momentum projection technique, to explain a variety of low- and high-spin phenomena in triaxial rotating nuclei.

  16. Effects of Λ hyperon on localization and clustering in p- and sd-shell nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Xu, Renli, E-mail: xurenli.phy@gmail.com [Key Laboratory of Modern Acoustics, Department of Physics, Nanjing University, Nanjing 210093 (China); Wu, Chen, E-mail: wuchenoffd@gmail.com [Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201800 (China); Ren, Zhongzhou, E-mail: zren@nju.edu.cn [Key Laboratory of Modern Acoustics, Department of Physics, Nanjing University, Nanjing 210093 (China); Center of Theoretical Nuclear Physics, National Laboratory of Heavy-Ion Accelerator, Lanzhou 730000 (China); Joint Center of Nuclear Science and Technology, Nanjing University, Nanjing 210093 (China)

    2015-01-15

    In the present work, the properties of several deformed p- and sd-shell Λ-hypernuclei have been investigated using the self-consistent relativistic mean field theory. The calculated ground state energies are consistent with the experimental values. In particular, the possibility of localization and clustering in deformed nuclei is discussed, concentrating on experimentally accessible light nuclei. Utilizing the framework of relativistic mean field model, our calculation predicts formation of clusterlike structure in the ground state of {sup 28}Si and {sup 32}S, while the core nuclei in {sup 29}{sub Λ}Si and {sup 33}{sub Λ}S show a delocalized formation in the presence hyperon depending on the nuclear effective interaction.

  17. VIRTUAL MASS EFFECT ON CONSTRAINED OSCILLATION OF OPEN SHELLS

    Directory of Open Access Journals (Sweden)

    Mr. Oleg Ye. Sysoyev  Doctor of Engineering, Professor, the Civil construction and Architecture Department, Dean of the Cadastre and Civil construction faculty, Komsomolsk-on-Amur State Technical University (Russia, Komsomolsk-on-Amur. E-mail: fks@knastu.ru.

    2016-09-01

    Full Text Available In the laboratory of constructions of Komsomolsk-on-Amur State Technical University (KnAGTU an experiment has been carried on. The aim of the experiment was to identify patterns of influence of magnitude of fluctuations in the virtual mass on constrained oscillation of open shells. Constrained oscillation of curved and open-shell carrying the virtual mass was measured with the help of induction accelerometers. Steel shell is pin supported along the edges, rectangular in the plan. Pin supported open shells along both sides, as the most frequently used in the construction have not yet been investigated. The calculation was made based on the general equation of oscillation of a shell, as well as Donnell - Mushtari - Vlasov equations. In the theoretical calculation, assumptions about the flatness were not taken into account. But it seemed that the magnitude of the stresses from bending moments are comparable in magnitude to the stress of the effort. In consequence, substantial increase in the differentiation was obtained. As a result, values of theoretical constrained oscillation of a shell were obtained. We compared the theoretical and analytical data.

  18. Measurements of M-Shell Dielectronic Recombination for Active Galactic Nuclei

    Science.gov (United States)

    Lukic, D.; Schnell, M.; Savin, D. W.; Mueller, A.; Schippers, S.; Schmidt, E. W.; Brandau, C.; Lestinsky, M.; Sprenger, F.; Wolf, A.

    2005-05-01

    XMM-Newton and Chandra spectroscopy of active galactic nuclei (AGNs) shows a rich spectrum of X-ray absorption lines. These AGN observations have detected a broad unresolved transition array (UTA) between 15-17 A. This is attributed to inner shell photoexcitation of M-shell iron. Modeling these UTA features is currently limited by uncertainties in the low temperature DR data for M-shell iron. In order to resolve this issue and to provide reliable iron M-shell DR data for plasma modeling, we are carrying out a series of laboratory measurements using the heavy-ion Test Storage Ring (TSR) at the Max-Plank-Institute for Nuclear Physics in Heidelberg, Germany. Other commonly used laboratory methods for studying DR (e.g., electron beam ion traps [EBITs]) are unable to measure the relevant low energy DR resonances. Storage rings are currently the only laboratory method capable of studying low temperature DR. We are also providing our data to atomic theorist to benchmark their modern DR calculations. Our initial results indicate that state-of-the-art theory cannot reliably predict the needed low temperature M-shell DR rate coefficients. Here we will report our recent results for DR of Fe XIV and Fe XIII and plans for future work. This work is supported part by NASA, the German Federal Ministry for Education and Research, and the German Research Council.

  19. Ab-initio take on effective single-particle energies in doubly closed shell nuclei

    CERN Document Server

    Duguet, T

    2011-01-01

    The present work discusses, from an ab-initio standpoint, the definition, the meaning, and the usefulness of effective single-particle energies (ESPEs) in doubly closed shell nuclei. We perform coupled-cluster calculations to quantify to what extent selected closed-shell nuclei in the oxygen and calcium isotopic chains can effectively be mapped onto an effective independent-particle picture. To do so, we revisit in detail the notion of ESPEs in the context of strongly correlated many-nucleon systems and illustrate the necessity to extract ESPEs through the diagonalization of the centroid {\\it matrix}, as originally argued by Baranger. For the purpose of illustration, we analyse the impact of correlations on observable one-nucleon separation energies and non-observable ESPEs in selected closed-shell oxygen and calcium isotopes. To further qualify the meaning and usefulness of ESPEs, we quantify the resolution-scale dependence of ESPEs and establish to what extent the first $2^+_1$ excitation energy is correlat...

  20. A novel approach to the systematization of α-decaying nuclei, based on shell structures

    Energy Technology Data Exchange (ETDEWEB)

    Yarman, Tolga; Azmi Altintas, Ali [Okan University, Istanbul (Turkey); Zaim, Nimet [Trakya University, Edirne (Turkey); Amon Susam, Lidya [Istanbul University, Istanbul (Turkey); Kholmetskii, Alexander [Belarus State University, Minsk (Belarus); Arik, Metin [Bogazici University, Istanbul (Turkey); Ozaydin, Fatih [Isik University, Istanbul (Turkey)

    2016-05-15

    We provide a novel systematization of α-decaying nuclei, starting with the classically adopted mechanism. The decay half-life of an α-disintegrating nucleus is framed, supposing that i) the α-particle is born inside the parent, then ii) it keeps on hitting the barrier, while it runs back and forth inside the parent, and hitting each time the barrier, and iii) it finally tunnels through the barrier. One can, knowing the decay half-life, consider the probability that the α-particle is born within the parent, before it is emitted, as a parameter. Under all circumstances, the decay appears to be governed by the shell structure of the given nucleus. Our approach well allows to incorporate (not only even-even nuclei, but) all nuclei, decaying via throwing an alpha particle. Though herein, we limit ourselves with just even-even nuclei, in the aim of comparing our results with the existing Geiger-Nuttal results. (orig.)

  1. Shell structure in neutron rich nuclei by means of binary reactions

    Energy Technology Data Exchange (ETDEWEB)

    Angelis, G. de [INFN, Laboratori Nazionali di Legnaro (Italy)

    2014-08-14

    Nuclear structure studies far from stability rely mainly on the availability of radioactive nuclear beams but can complementary be addressed by means of high intensity beams of stable ions. In such contest, deep-inelastic and multinucleon transfer reactions are a powerful tool to populate yrast and non yrast states in neutron-rich nuclei. Particularly successful is here the combination of large acceptance spectrometers with highly segmented gamma-detector arrays. Such devices can provide the necessary channel selectivity to identify very rare signals. The AGATA gamma-ray detector array coupled to the PRISMA spectrometer at the Legnaro National Laboratories (LNL) in Italy is one example. Large data sets have been collected at LNL for nuclei close to the N=20, 28, 40, 50 and 82 shell closures.

  2. Origin of fine structure of the giant dipole resonance in sd-shell nuclei

    CERN Document Server

    Fearick, R W; Matsubara, H; von Neumann-Cosel, P; Richter, A; Roth, R; Tamii, A

    2014-01-01

    A set of high resolution zero-degree inelastic proton scattering data on 24Mg, 28Si, 32S, and 40Ca provides new insight into the long-standing puzzle of the origin of fragmentation of the Giant Dipole Resonance (GDR) in sd-shell nuclei. Understanding is provided by state-of-the-art theoretical Random Phase Approximation (RPA) calculatios for deformed nuclei using for the first time a realistic nucleon-nucleon interaction derived from the Argonne V18 potential with the unitary correlation operator method and supplemented by a phenomenological three-nucleon contact interaction. A wavelet analysis allows to extract significant scales both in the data and calculations characterizing the fine structure of the GDR. The fair agreement supports that the fine structure arises from ground-state deformation driven by alpha clustering.

  3. Branching Ratios of a Decay for Nuclei near Deformed Shell Closures

    Institute of Scientific and Technical Information of China (English)

    WANG Yan-Zhao; ZHANG Hong-Fei; DONG Jian-Min; SU Xin-Ning; ZUO Wei; LI Jun-Qing

    2009-01-01

    The generalized liquid drop model (GLDM) is extended to the region around deformed shell closure 270Hs by taking into account the excitation energy EI+ of the residual daughter nucleus and the centrifugal potential energy Vcen(r).The branching ratios of a decays from the ground state of a parent nucleus to the ground state 0+ of its deformed daughter nucleus and to the first excited state 2+ are calculated in the framework of the GLDM.The results support the proposal that a measurement of α spectroscopy is a feasible method to extract information on nuclear deformation of superheavy nuclei around the deformed nucleus 270 Hs.

  4. Study of the Doubly-closed Shell Nucleus $^{132}$Sn and its Valence Nuclei

    CERN Multimedia

    2002-01-01

    The aim of the experiment is to study the level structure of nuclei close to the shell closures (Z,N)~=~(50,50) and (50,82). \\\\ \\\\ The decay of the isotopes |9|8Cd, |1|3|2In, |1|3|3In and|1|3|1Cd are invesigated by means of $\\gamma$; electron- and neutron spectroscopy. Gamma-gamma and electron-gamma coincidences are also recorded.\\\\ \\\\ The experimental equipment (Ge(Li) detectors, Si(Li) detectors and |3He neutron spectrometers) are connected on-line to the ISOLDE on-line isotope separator.

  5. Evidence for Symplectic Symmetry in Ab Initio No-Core Shell Model Results for Light Nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Dytrych, Tomas; Sviratcheva, Kristina D.; Bahri, Chairul; Draayer, Jerry P.; /Louisiana State U.; Vary, James P.; /Iowa State U. /LLNL, Livermore /SLAC

    2007-04-24

    Clear evidence for symplectic symmetry in low-lying states of {sup 12}C and {sup 16}O is reported. Eigenstates of {sup 12}C and {sup 16}O, determined within the framework of the no-core shell model using the JISP16 NN realistic interaction, typically project at the 85-90% level onto a few of the most deformed symplectic basis states that span only a small fraction of the full model space. The results are nearly independent of whether the bare or renormalized effective interactions are used in the analysis. The outcome confirms Elliott's SU(3) model which underpins the symplectic scheme, and above all, points to the relevance of a symplectic no-core shell model that can reproduce experimental B(E2) values without effective charges as well as deformed spatial modes associated with clustering phenomena in nuclei.

  6. Influence of proton shell closure on the evaporation residue cross sections of superheavy nuclei

    Science.gov (United States)

    Bao, X. J.; Guo, S. Q.; Zhang, H. F.; Li, J. Q.

    2017-04-01

    Within the dinuclear system model we systematically calculate the evaporation residue cross sections (ERCSs) of superheavy nuclei (SHN) for the 48Ca-induced hot fusion reactions. Different calculations of the fission barriers of the SHN are used. The difference is as large as two orders of magnitude of ERCSs by applying the various fission barriers for the reaction 48Ca+249Cf. The dependence of the calculated ERCSs on the predicted shell structure and magic numbers of the heavier SHN is discussed. It is found that the structure of SHN crucially influences the ERCSs. Measurement of ERCSs for at least one isotope of the Z > 118 nucleus would help us to set a proper shell model for the SHN with Z > 118.

  7. K -shell ionization during α decay of polonium isotopes and superheavy nuclei

    Science.gov (United States)

    Trzhaskovskaya, M. B.; Nikulin, V. K.

    2016-03-01

    The theory of K -shell ionization during α decay of the 84Po isotopes is considered in detail as a part of our general study of the inner shell ionization probability of heavy and superheavy nuclei. Calculations of K -shell ionization with allowance made for the α -particle tunneling through the atomic Coulomb barrier have been performed in the framework of the fully quantum mechanical treatment developed for the first time by Anholt and Amundsen. Further information is available [Anholt and Amundsen, Phys. Rev. A 25, 169 (1982), 10.1103/PhysRevA.25.169]. As distinct from all previous the K -shell ionization calculations where the Dirac hydrogenlike wave functions have been used, we have found the discrete and continuum electron wave functions in the framework of the relativistic self-consistent Dirac-Fock method. In addition, we have taken into consideration accurately terms associated with the α -particle tunneling. Our exact calculations show that the tunneling contribution to the ionization probability is of great importance while Anholt and Amundsen have asserted that the contribution is small. We have obtained that the K -shell ionization probability during α decay of five isotopes of 84Po correlate better with the available experimental data providing the tunneling is included in calculations. New calculations for K -shell ionization during α decay of superheavy elements Fm249100,No253102,Rg272111, as well as Rn22286 are also presented. The data may be of importance in the combined α ,γ , and conversion-electron spectroscopy used in the superheavy element synthesis analysis.

  8. Microscopic calculations of C2 and C4 form factors in sd-shell nuclei

    CERN Document Server

    Radhi, R A

    2003-01-01

    Inelastic electron scattering to 2 sup + and 4 sup + states for the even-even N=Z sd-shell nuclei ( sup 2 sup 0 Ne, sup 2 sup 4 Mg, sup 2 sup 8 Si and sup 3 sup 2 S) are discussed taking into account higher energy configurations outside the sd-shell. Higher energy configurations, which are called core polarization effects, are included through a microscopic theory that includes excitations from the core 1s and 1p orbits and also from 2s-1d shell to the higher allowed orbits with 2 Planck constant omega excitations. The predictions of C2 and C4 Coulomb form factors are compared with the available experimental data. The calculations based on the Wildenthal interaction for the sd-shell model space and on the modified surface delta interaction for the core-polarization effects. The effect of higher excited configurations is found essential in both the transition strength and momentum transfer dependence of form factors, and gives a remarkably good agreement with the measured data.

  9. Light Nuclei in the Framework of the Symplectic No-Core Shell Model

    Energy Technology Data Exchange (ETDEWEB)

    Draayer, Jerry P.; Dytrych, Tomas; Sviratcheva, Kristina D.; Bahri, Chairul; /Louisiana State U.; Vary, James P.; /Iowa State U. /LLNL, Livermore /SLAC

    2007-04-02

    A symplectic no-core shell model (Sp-NCSM) is constructed with the goal of extending the ab-initio NCSM to include strongly deformed higher-oscillator-shell configurations and to reach heavier nuclei that cannot be studied currently because the spaces encountered are too large to handle, even with the best of modern-day computers. This goal is achieved by integrating two powerful concepts: the ab-initio NCSM with that of the Sp(3,R) {contains} SU(3) group-theoretical approach. The NCSM uses modern realistic nuclear interactions in model spaces that consists of many-body configurations up to a given number of {h_bar}{Upsilon} excitations together with modern high-performance parallel computing techniques. The symplectic theory extends this picture by recognizing that when deformed configurations dominate, which they often do, the model space can be better selected so less relevant low-lying {h_bar}{Upsilon} configurations yield to more relevant high-lying {h_bar}{Upsilon} configurations, ones that respect a near symplectic symmetry found in the Hamiltonian. Results from an application of the Sp-NCSM to light nuclei are compared with those for the NCSM and with experiment.

  10. Shell model method for Gamow-Teller Transitions in heavy, deformed nuclei

    CERN Document Server

    Gao, Z C; Sun, Y; Gao, Zao-Chun; Sun, Yang

    2006-01-01

    A method for calculation of Gamow-Teller transition rates is developed by using the concept of the Projected Shell Model (PSM). The shell model basis is constructed by superimposing angular-momentum-projected multi-quasiparticle configurations, and nuclear wave functions are obtained by digonalizing the two-body interactions in these projected states. Calculation of transition matrix elements in the PSM framework is discussed in detail, and the effects caused by the Gamow-Teller residual forces and by configuration-mixing are studied. With this method, it may become possible to perform a state-by-state calculation for beta-decay and electron-capture rates in heavy, deformed nuclei at finite temperatures. Our first example indicates that, while experimentally known Gamow-Teller transition rates from the ground state of the parent nucleus are reproduced, stronger transitions from some low-lying excited states are predicted to occur, which may considerably enhance the total decay rates once these nuclei are expo...

  11. Differences in neurogenesis differentiate between core and shell regions of auditory nuclei in the turtle (Pelodiscus sinensis): evolutionary implications.

    Science.gov (United States)

    Zeng, Shao-Ju; Xi, Chao; Zhang, Xin-Wen; Zuo, Ming-Xue

    2007-01-01

    There is a clear core-versus-shell distinction in cytoarchitecture, electrophysiological properties and neural connections in the mesencephalic and diencephalic auditory nuclei of amniotes. Determining whether the embryogenesis of auditory nuclei shows a similar organization is helpful for further understanding the constituent organization and evolution of auditory nuclei. Therefore in the present study, we injected [(3)H]-thymidine into turtle embryos (Pelodiscus sinensis) at various stages of development. Upon hatching, [(3)H]-thymidine labeling was examined in both the core and shell auditory regions in the midbrain, diencephalon and dorsal ventricular ridge. Met-enkephalin and substance P immunohistochemistry was used to distinguish the core and shell regions. In the mesencephalic auditory nucleus, the occurrence of heavily labeled neurons in the nucleus centralis of the torus semicircularis reached its peak at embryonic day 9, one day later than the surrounding shell. In the diencephalic auditory nucleus, the production of heavily labeled neurons in the central region of the reuniens (Re) was highest at embryonic day (E) 8, one day later than that in the shell region of reuniens. In the region of the dorsal ventricular ridge that received inputs from the central region of Re, the appearance of heavily labeled neurons also reached a peak one day later than that in the area receiving inputs from the shell region of reuniens. Thus, there is a core-versus-shell organization of neuronal generation in reptilian auditory areas. Copyright (c) 2007 S. Karger AG, Basel.

  12. Linking partial and quasi dynamical symmetries in rotational nuclei and shell evolution in {sup 96}Zr

    Energy Technology Data Exchange (ETDEWEB)

    Kremer, Christoph

    2016-01-27

    The first part of this thesis revolves around symmetries in the sd-IBA-1. A region of approximate O(6) symmetry for the ground-state band, a partial dynamical symmetry (PDS) of type III, in the parameter space of the extended consistent-Q formalism is identified through quantum number fluctuations. The simultaneous occurrence of a SU(3) quasi dynamical symmetry for nuclei in the region of O(6) PDS is explained via the β=1, γ=0 intrinsic state underlying the ground-state band. The previously unrelated concepts of PDS and QDS are connected for the first time and many nuclei in the rare earth region that approximately satisfy both symmetry requirements are identified. Ground-state to ground-state (p, t) transfer reactions are presented as an experimental signature to identify pairs of nuclei that both exhibit O(6) PDS. In the second part of this thesis inelastic electron scattering off {sup 96}Zr is studied. The experiment was performed at the high resolution Lintott spectrometer at the S-DALINAC and covered a momentum-transfer range of 0.28 - 0.59 fm{sup -1}. Through a relative analysis using Plane Wave Born Approximation (PWBA) the B(E2;2{sup +}{sub 2}→0{sup +}{sub 1}) value is extracted without incurring the additional model dependence of a Distorted Wave Born Approximation (DWBA). By combining this result with known multipole mixing ratios and branching ratios all decay strengths of the 2{sup +}{sub 2} state are determined. A mixing calculation establishes very weak mixing (V{sub mix}=76 keV) between states of the ground-state band and those of the band build on top of the 0{sup +}{sub 2} state which includes the 2{sup +}{sub 2} state. The occurrence of these two isolated bands is interpreted within the shell model in terms of type II shell evolution.

  13. Microscopic description of quadrupole collectivity in neutron-rich nuclei across the N = 126 shell closure

    Energy Technology Data Exchange (ETDEWEB)

    Rodriguez-Guzman, R.; Sharma, M.M. [Kuwait University, Physics Department, Kuwait (Kuwait); Robledo, L.M. [Universidad Autonoma de Madrid, Departamento de Fisica Teorica, Madrid (Spain)

    2015-06-15

    The quadrupole collectivity in Nd, Sm, Gd, Dy, Er, Yb, Hf and W nuclei with neutron numbers 122 ≤ N ≤ 156 is studied, both at the mean field level and beyond, using the Gogny energy density functional. Besides the robustness of the N = 126 neutron shell closure, it is shown that the onset of static deformations in those isotopic chains with increasing neutron number leads to an enhanced stability and further extends the corresponding two-neutron drip lines far beyond what could be expected from spherical calculations. Independence of the mean-field predictions with respect to the particular version of the Gogny energy density functional employed is demonstrated by comparing results based on the D1S and D1M parameter sets. Correlations beyond mean field are taken into account in the framework of the angular momentum projected generator coordinate method calculation. It is shown that N = 126 remains a robust neutron magic number when dynamical effects are included. The analysis of the collective wave functions, average deformations and excitation energies indicate that, with increasing neutron number, the zero-point quantum corrections lead to dominant prolate configurations in the 0{sub 1} {sup +}, 0{sub 2} {sup +}, 2{sub 1} {sup +} and 2{sub 2} {sup +} states of the studied nuclei. Moreover, those dynamical deformation effects provide an enhanced stability that further supports the mean-field predictions, corroborating a shift of the r-process path to higher neutron numbers. Beyond mean-field calculations provide a smaller shell gap at N = 126 than the mean-field one in good agreement with previous theoretical studies. However, the shell gap still remains strong enough in the two-neutron drip lines. (orig.)

  14. Effectively-truncated large-scale shell-model calculations and nuclei around 100Sn

    Science.gov (United States)

    Gargano, A.; Coraggio, L.; Itaco, N.

    2017-09-01

    This paper presents a short overview of a procedure we have recently introduced, dubbed the double-step truncation method, which is aimed to reduce the computational complexity of large-scale shell-model calculations. Within this procedure, one starts with a realistic shell-model Hamiltonian defined in a large model space, and then, by analyzing the effective single particle energies of this Hamiltonian as a function of the number of valence protons and/or neutrons, reduced model spaces are identified containing only the single-particle orbitals relevant to the description of the spectroscopic properties of a certain class of nuclei. As a final step, new effective shell-model Hamiltonians defined within the reduced model spaces are derived by way of a unitary transformation of the original large-scale Hamiltonian. A detailed account of this transformation is given and the merit of the double-step truncation method is illustrated by discussing few selected results for 96Mo, described as four protons and four neutrons outside 88Sr. Some new preliminary results for light odd-tin isotopes from A = 101 to 107 are also reported.

  15. Equivalence between local Fermi gas and shell models in inclusive muon capture from nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Amaro, J.E.; Nieves, J.; Valverde, M. [Universidad de Granada, Departamento de Fisica Moderna, Granada (Spain); Maieron, C. [INFN, Sezione di Catania, Catania (Italy)

    2005-06-01

    Motivated by recent studies of inclusive neutrino nucleus processes and muon capture within a correlated local Fermi gas model (LFG), we discuss the relevance of nuclear finite-size effects in these reactions at low energy, in particular for muon capture. To disentangle these effects from others coming from the reaction dynamics we employ here a simple uncorrelated shell model that embodies the typical finite-size content of the problem. The integrated decay widths of muon atoms calculated with this shell model are then compared for several nuclei with those obtained within the uncorrelated LFG, using in both models exactly the same theoretical ingredients and parameters. We find that the two predictions are in quite good agreement, within 1-7%, when the shell model density and the correct energy balance is used as input in the LFG calculation. The present study indicates that, despite the low excitation energies involved in the reaction, integrated inclusive observables, like the total muon capture width, are quite independent of the fine details of the nuclear wave functions. (orig.)

  16. Spectroscopy of 70Kr and isospin symmetry in the T =1 f p g shell nuclei

    Science.gov (United States)

    Debenham, D. M.; Bentley, M. A.; Davies, P. J.; Haylett, T.; Jenkins, D. G.; Joshi, P.; Sinclair, L. F.; Wadsworth, R.; Ruotsalainen, P.; Henderson, J.; Kaneko, K.; Auranen, K.; Badran, H.; Grahn, T.; Greenlees, P.; HerzaáÅ, A.; Jakobsson, U.; Konki, J.; Julin, R.; Juutinen, S.; Leino, M.; Sorri, J.; Pakarinen, J.; Papadakis, P.; Peura, P.; Partanen, J.; Rahkila, P.; Sandzelius, M.; Sarén, J.; Scholey, C.; Stolze, S.; Uusitalo, J.; David, H. M.; de Angelis, G.; Korten, W.; Lotay, G.; Mallaburn, M.; Sahin, E.

    2016-11-01

    The recoil-β tagging technique has been used in conjunction with the 40Ca(32S,2 n ) reaction at a beam energy of 88 MeV to identify transitions associated with the decay of the 2+ and, tentatively, 4+ states in the nucleus 70Kr. These data are used, along with previously published data, to examine the triplet energy differences (TED) for the mass 70 isobars. The experimental TED values are compared with shell model calculations, performed with the JUN45 interaction in the f p g model space, that include a J =0 isospin nonconserving (INC) interaction with an isotensor strength of 100 keV. The agreement is found to be very good up to spin 4 and supports the expectation for analog states that all three nuclei have the same oblate shape at low-spin. The A =70 results are compared with the experimental and shell model predicted TED and mirror energy differences (MED) for the mass 66 and 74 systems. The comparisons clearly demonstrate the importance of the isotensor INC interaction in replicating the TED data in this region. Issues related to the observed MED values and their interpretation within the shell model are discussed.

  17. Intermediate-energy inverse-kinematics one-proton pickup reactions on neutron-deficient $fp$-shell nuclei

    CERN Document Server

    McDaniel, S; Tostevin, J A; Baugher, T; Bazin, D; Brown, B A; Cook, J M; Glasmacher, T; Grinyer, G F; Ratkiewicz, A; Weisshaar, D

    2012-01-01

    Background: Thick-target-induced nucleon-adding transfer reactions onto energetic rare-isotope beams are an emerging spectroscopic tool. Their sensitivity to single-particle structure complements one-nucleon removal reaction capabilities in the quest to reveal the evolution of nuclear shell structure in very exotic nuclei. Purpose: To add intermediate-energy, carbon-target-induced one-proton pickup reactions to the arsenal of $\\gamma$-ray tagged direct reactions applicable in the regime of low beam intensities and to apply these for the first time to $fp$-shell nuclei. Methods: Inclusive and partial cross sections were measured for the $\

  18. Recombination of open-f-shell tungsten ions

    Science.gov (United States)

    Krantz, C.; Badnell, N. R.; Müller, A.; Schippers, S.; Wolf, A.

    2017-03-01

    We review experimental and theoretical efforts aimed at a detailed understanding of the recombination of electrons with highly charged tungsten ions characterised by an open 4f sub-shell. Highly charged tungsten occurs as a plasma contaminant in ITER-like tokamak experiments, where it acts as an unwanted cooling agent. Modelling of the charge state populations in a plasma requires reliable thermal rate coefficients for charge-changing electron collisions. The electron recombination of medium-charged tungsten species with open 4f sub-shells is especially challenging to compute reliably. Storage-ring experiments have been conducted that yielded recombination rate coefficients at high energy resolution and well-understood systematics. Significant deviations compared to simplified, but prevalent, computational models have been found. A new class of ab initio numerical calculations has been developed that provides reliable predictions of the total plasma recombination rate coefficients for these ions.

  19. Shell Model Predictions for Very Neutron-Rich Nuclei in 132SN Region Interesting Features of Effective- Charge Revealed

    CERN Document Server

    Sarkar, S; Sarkar, Sukhendusekhar

    2005-01-01

    Shell model studies have been done for very neutron - rich nuclei in the range Z=50-55 and N=82-87. Good agreement of the theoretical level spectra with the experimental one for N=82, 83 I and Te nuclei is shown. Then the results for three very neutron-rich nuclei 137Sn and 136-137Sb have been presented. The present calculation favour a 2- ground state for 136Sb instead of 1- identified through beta decay.Interesting observation about the E2 effective charges for this region has been discussed.

  20. Shell-model half-lives for r-process waiting point nuclei including first-forbidden contributions

    CERN Document Server

    Zhi, Q; Cuenca-García, J J; Langanke, K; Martínez-Pinedo, G; Sieja, K

    2013-01-01

    We have performed large-scale shell-model calculations of the half-lives and neutron-branching probabilities of the r-process waiting point nuclei at the magic neutron numbers N=50, 82, and 126. The calculations include contributions from allowed Gamow-Teller and first-forbidden transitions. We find good agreement with the measured half-lives for the N=50 nuclei with charge numbers Z=28-32 and for the N=82 nuclei 129Ag and 130Cd. The contribution of forbidden transitions reduce the half-lives of the N=126 waiting point nuclei significantly, while they have only a small effect on the half-lives of the N=50 and 82 r-process nuclei.

  1. Shell model yrast states in the N=79 nuclei [sup 141]Sm and [sup 143]Gd

    Energy Technology Data Exchange (ETDEWEB)

    Lach, M. (Institut fuer Kernphysik, Forschungszentrum Juelich (Germany)); Kleinheinz, P. (Institut fuer Kernphysik, Forschungszentrum Juelich (Germany)); Blomqvist, J. (Manne Siegbahninstitutet foer Fysik, Stockholm (Sweden)); Ercan, A. (Institut fuer Kernphysik, Forschungszentrum Juelich (Germany)); Haehn, H.J. (Institut fuer Kernphysik, Forschungszentrum Juelich (Germany)); Wahner, D. (Institut fuer Kernphysik, Forschungszentrum Juelich (Germany)); Julin, R. (Institut fuer Kernphysik, Forschungszentrum Juelich (Germany)); Zupancic, M. (Institut fuer Kernphysik, Forschungszentrum Juelich (Germany)); Cigoroglu, F. (Institut fuer Kernphysik, Forschungszentrum Juelich (Germany)); De Angelis, G.

    1993-06-01

    In ([alpha],5n) in-beam [gamma]- and electron measurements we have established high-spin states in the 3-neutronhole nuclei [sup 141]Sm and [sup 143]Gd. Observed energy levels below 4 MeV are interpreted in terms of shell model configurations where the odd h[sub 11/2] neutron hole couples to the N=80 core excitations containing one h[sub 11/2] proton particle or one h[sub 11/2] neutron hole. Higher-lying yrast states are built on a 23/2[sup -] level at approx 3.2 MeV probably involving the [pi]h[sup 2][sub 11/2][nu]h[sup -1][sub 11/2] configuration. (orig.)

  2. Spectroscopy of Neutron-Deficient Nuclei Near the Z=82 Closed Shell via Symmetric Fusion Reactions

    Directory of Open Access Journals (Sweden)

    Kondev F.G.

    2013-12-01

    Full Text Available In-beam and decay-spectroscopy studies of neutron-deficient nuclei near the Z=82 shell closure were carried out using the Fragment Mass Analyzer (FMA and the Gammasphere array, in conjunction with symmetric fusion reactions and the Recoil Decay Tagging (RDT technique. The primary motivation was to study properties of 179Tl and 180Tl, and their daughter, and grand-daughter isotopes. For the first time, in-beam structures associated with 179Tl and 180Tl were observed, as well as γ rays associated with the 180Tl α decay. No long-lived isomer was identified in 180Tl, in contrast with the known systematics for the heavier odd-odd Tl isotopes.

  3. Effective Interactions and Operators in Nuclei within the No-Core Shell Model

    Energy Technology Data Exchange (ETDEWEB)

    Barrett, B; Navratil, P; Stetcu, I; Vary, J

    2005-09-14

    We review the application of effective operator formalism to the ab initio no core shell model (NCSM). For short-range operators, such as the nucleon-nucleon potential, the unitary-transformation method works extremely well at the two-body cluster approximation and good results are obtained for the binding energies and excitation spectra of light nuclei (A {<=} 16). However, for long-range operators, such as the radius or the quadrupole moment, performing this unitary transformation at the two-body cluster level, does not include the higher-order correlations needed to renormalize these long-range operators adequately. Usually, such correlations can be obtained either by increasing the order of the cluster approximation, or by increasing the model space. We will discuss the difficulties of these approaches as well as alternate possible solutions for including higher-order correlations in small model spaces.

  4. Quasi-SU(3) truncation scheme for even-even sd-shell nuclei

    CERN Document Server

    Vargas, C E; Draayer, J P

    2000-01-01

    The Quasi-SU(3) symmetry was uncovered in full pf and sdg shell-model calculations for both even-even and odd-even nuclei. It manifests itself through a dominance of single-particle and quadrupole-quadrupole terms in the Hamiltonian used to describe well-deformed nuclei. A practical consequence of the quasi-SU(3) symmetry is an efficient basis truncation scheme. In a recent work was shown that when this type of Hamiltonian is diagonalized in an SU(3) basis, only a few irreducible represntations (irreps) of SU(3) are needed to describe the Yrast band, the leading S = 0 irrep augmented with the leading S = 1 irreps in the proton and neutron subspaces. In the present article the quasi-SU(3) truncation scheme is used, in conjunction with a "realistic but schematic" Hamiltonian that includes the most important multipole terms, to describe the energy spectra and B(E2) transition strengths of 20-Ne, 22-Ne, 24-Mg and 28-Si. The effect of the size of the Hilbert space on both sets of observables is discussed, as well ...

  5. Shell model based reaction rates for rp-process nuclei in the mass range A=44-63

    CERN Document Server

    Fisker, J L; Görres, J; Langanke, K; Martínez-Pinedo, G; Wiescher, M C

    2001-01-01

    We have used large-scale shell-model diagonalization calculations to determine the level spectra, proton spectroscopic factors, and electromagnetic transition probabilities for proton rich nuclei in the mass range A=44-63. Based on these results and the available experimental data, we calculated the resonances for proton capture reactions on neutron deficient nuclei in this mass range. We also calculated the direct capture processes on these nuclei in the framework of a Woods-Saxon potential model. Taking into account both resonant and direct contributions, we determined the ground-state proton capture reaction rates for these nuclei under hot hydrogen burning conditions for temperatures between 10 sup 8 and 10 sup 1 sup 0 K. The calculated compound-nucleus level properties and the reaction rates are presented here; the rates are also available in computer-readable format from the authors.

  6. How nuclei of Giardia pass through cell differentiation: semi-open mitosis followed by nuclear interconnection.

    Science.gov (United States)

    Jiráková, Klára; Kulda, Jaroslav; Nohýnková, Eva

    2012-05-01

    Differentiation into infectious cysts (encystation) and multiplication of pathogenic trophozoites after hatching from the cyst (excystation) are fundamental processes in the life cycle of the human intestinal parasite Giardia intestinalis. During encystation, a bi-nucleated trophozoite transforms to a dormant tetra-nucleated cyst enveloped by a protective cyst wall. Nuclear division during encystation is not followed by cytokinesis. In contrast to the well-studied mechanism of cyst wall formation, information on nuclei behavior is incomplete and basic cytological data are lacking. Here we present evidence that (1) the nuclei divide by semi-open mitosis during early encystment; (2) the daughter nuclei coming from different parent nuclei are always arranged in pairs; (3) in both pairs, the nuclei are interconnected via bridges formed by fusion of their nuclear envelopes; (4) each interconnected nuclear pair is associated with one basal body tetrad of the undivided diplomonad mastigont; and (5) the interconnection between nuclei persists through the cyst stage being a characteristic feature of encysted Giardia. Based on the presented results, a model of nuclei behavior during Giardia differentiation is proposed.

  7. Nuclear shell effects in neutron-rich nuclei around N=20 and N=32,34

    CERN Document Server

    Seidlitz, M

    Nuclear shell effects in neutron-rich nuclei around N=20 and N=32,34 were studied by means of reduced transition probabilities, i.e. B(E2) and B(M1) values. To this end a series of Coulomb-excitation experiments, employing radioactive 31Mg and 29,30Na beams, as well as a precise lifetime experiment of excited states in 56Cr were performed. The collective properties of excited states of 31Mg were the subject of a Coulomb-excitation experiment at REX-ISOLDE, CERN, employing a radioactive 31Mg beam at a beam energy of 3.0 MeV/u. The beam intensity amounted to 3000 ions/s on average. The highly efficient MINIBALL setup was employed, consisting of eight HPGe cluster detectors for gamma-ray detection and a segmented Si-detector for coincident particle detection. The level scheme of 31Mg was extended. Spin and parity assignment of the observed 945 keV state yielded 5/2+ and its de-excitation is dominated by a strong collective M1 transition. Comparison of the transition probabilities of 30,31,32Mg establishes that f...

  8. Description of collective and quasiparticle excitations in deformed actinide nuclei: The first application of the Heavy Shell Model

    CERN Document Server

    Cui, Ji-Wei; Chen, Fang-Qi; Sun, Yang; Wu, Cheng-Li; Gao, Zao-Chun

    2014-01-01

    The Heavy Shell Model (HSM) (Y. Sun and C.-L. Wu, Phys. Rev. C 68, 024315 (2003)) was proposed to take the advantages of two existing models, the projected shell model (PSM) and the Fermion Dynamical Symmetry Model (FDSM). To construct HSM, one extends the PSM by adding collective D-pairs into the intrinsic basis. The HSM is expected to describe simultaneously low-lying collective and quasi-particle excitations in deformed nuclei, and still keeps the model space tractable even for the heaviest systems. As the first numerical realization of the HSM, we study systematically the band structures for some deformed actinide nuclei, with a model space including up to 4-quasiparticle and 1-D-pair configurations. The calculated energy levels for the ground- state bands, the collective bands such as {\\beta} - and {\\gamma} -bands, and some quasiparticle bands agree well with known experimental data. Some low-lying quasiparticle bands are predicted, awaiting experimental confirmation.

  9. Electron recombination with tungsten ions with open f-shells

    CERN Document Server

    Harabati, C; Flambaum, V V; Dzuba, V A

    2016-01-01

    We calculate the electron recombination rates with target ions W$^{q+}$, $q = 18$ -- $25$, as functions of electron energy and electron temperature (i.e. the rates integrated over the Maxwellian velocity distribution). Comparison with available experimental data for W$^{18+}$, W$^{19+}$, and W$^{20+}$ is used as a test of our calculations. Our predictions for W$^{21+}$, W$^{22+}$, W$^{23+}$, W$^{24+}$, and W$^{25+}$ (where the experimental data are not available) may be used for plasma modelling in thermonuclear reactors. All of these ions have an open electron $f$-shell and have an extremely dense spectrum of chaotic many-electron compound resonances which enhance the recombination rates by 2-3 orders of magnitude in comparison with the direct electron recombination. Conventional dielectronic recombination theory is not directly applicable in this case. Instead, we developed a statistical theory based on the properties of chaotic eigenstates. This theory describes a multi-electronic recombination (extension ...

  10. Deuteron-induced nucleon transfer reactions within an ab initio framework: First application to p-shell nuclei

    CERN Document Server

    Raimondi, Francesco; Navrátil, Petr; Quaglioni, Sofia

    2016-01-01

    Background: Low-energy transfer reactions in which a proton is stripped from a deuteron projectile and dropped into a target play a crucial role in the formation of nuclei in both primordial and stellar nucleosynthesis, as well as in the study of exotic nuclei using radioactive beam facilities and inverse kinematics. Ab initio approaches have been successfully applied to describe the $^3$H$(d,n)^4$He and $^3$He$(d,p)^4$He fusion processes. Purpose: An ab initio treatment of transfer reactions would also be desirable for heavier targets. In this work, we extend the ab initio description of $(d,p)$ reactions to processes with light $p$-shell nuclei. As a first application, we study the elastic scattering of deuterium on $^7$Li and the ${}^{7}$Li($d$,$p$)${}^{8}$Li transfer reaction based on a two-body Hamiltonian. Methods: We use the no-core shell model to compute the wave functions of the nuclei involved in the reaction, and describe the dynamics between targets and projectiles with the help of microscopic-clu...

  11. Coulomb energy difference as a probe of isospin-symmetry breaking in the upper fp-shell nuclei

    CERN Document Server

    Kaneko, K; Sun, Y; Tazaki, S; de Angelis, G

    2012-01-01

    The anomaly in Coulomb energy differences (CED) between the isospin T=1 states in the odd-odd N=Z nucleus 70Br and the analogue states in its even-even partner 70Se has remained a puzzle. This is a direct manifestation of isospin-symmetry breaking in effective nuclear interactions. Here, we perform large-scale shell-model calculations for nuclei with A=66-78 using the new filter diagonalization method based on the Sakurai-Sugiura algorithm. The calculations reproduce well the experimental CED. The observed negative CED for A=70 are accounted for by the cross-shell neutron excitations from the fp-shell to the g9/2 intruder orbit with the enhanced electromagnetic spin-orbit contribution at this special nucleon number.

  12. Deuteron-induced nucleon transfer reactions within an ab initio framework: First application to p -shell nuclei

    Science.gov (United States)

    Raimondi, Francesco; Hupin, Guillaume; Navrátil, Petr; Quaglioni, Sofia

    2016-05-01

    Background: Low-energy transfer reactions in which a proton is stripped from a deuteron projectile and dropped into a target play a crucial role in the formation of nuclei in both primordial and stellar nucleosynthesis, as well as in the study of exotic nuclei using radioactive beam facilities and inverse kinematics. Ab initio approaches have been successfully applied to describe the 3H (d ,n )4He and 3He(d ,p )4He fusion processes. Purpose: An ab initio treatment of transfer reactions would also be desirable for heavier targets. In this work, we extend the ab initio description of (d ,p ) reactions to processes with light p -shell nuclei. As a first application, we study the elastic scattering of deuterium on 7Li and the 7Li(d ,p )8Li transfer reaction based on a two-body Hamiltonian. Methods: We use the no-core shell model to compute the wave functions of the nuclei involved in the reaction, and describe the dynamics between targets and projectiles with the help of microscopic-cluster states in the spirit of the resonating group method. Results: The shapes of the excitation functions for deuterons impinging on 7Li are qualitatively reproduced up to the deuteron breakup energy. The interplay between d -7Li and p -8Li particle-decay channels determines some features of the 9Be spectrum above the d +7Li threshold. Our prediction for the parity of the 17.298 MeV resonance is at odds with the experimental assignment. Conclusions: Deuteron stripping reactions with p -shell targets can now be computed ab initio, but calculations are very demanding. A quantitative description of the 7Li(d ,p )8Li reaction will require further work to include the effect of three-nucleon forces and additional decay channels and to improve the convergence rate of our calculations.

  13. Electron-impact excitation of open d-shell ions

    Science.gov (United States)

    Ramsbottom, C. A.; Ballance, C. P.; Hibbert, A.; Keenan, F. P.

    2015-09-01

    Astrophysics is driven by observations, and in the present era there are a wealth of state-of-the-art ground-based and satellite facilities. The astrophysical spectra emerging from these are of exceptional quality and quantity and cover a broad wavelength range. To meaningfully interpret these spectra, astronomers employ highly complex modelling codes to simulate the astrophysical observations. Important input to these codes include atomic data such as excitation rates, photoionization cross sections, oscillator strengths, transition probabilities and energy levels/line wavelengths. Due to the relatively low temperatures associated with many astrophysical plasmas, the accurate determination of electron-impact excitation rates in the low energy region is essential in generating a reliable spectral synthesis. Hence it is these atomic data, and the main computational methods used to evaluate them, which we focus on in this publication. We consider in particular the complicated open d- shell structures of the Fe-peak ions in low ionization stages. While some of these data can be obtained experimentally, they are usually of insufficient accuracy or limited to a small number of transitions.

  14. Deformed optical potential anomaly in {open_quotes}soft{close_quotes} nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Lubian, J.; Cabezas, R. [Center for Applied Studies to Nuclear Development, Havana (Cuba)

    1994-12-31

    An analysis of the low-energy neutron inelastic scattering in some {open_quotes}soft{close_quotes} nuclei is made in the region of medium atomic-weight nuclei. A combined use of the coupled channel method (CCM) and statistical Hauser-Feshbach theory is applied. As structural model of the target nucleus in the CCM calculation the Davydov-Chaban model (DCM) is used. It is observed that the lineal coefficient of the real part energy dependence of the deformed optical potential becomes unusual and increase with the {open_quotes}softness{close_quotes} of the nucleus. It is shown that in the frame of the DCM it is possible to describe adequately experimental differential, integral and total cross sections in the energy range 1-5 MeV and the structure of the low-lying collective states.

  15. Multi-phonon gamma-vibrational bands in odd-mass nuclei studied by triaxial projected shell model approach

    Energy Technology Data Exchange (ETDEWEB)

    Sheikh, J.A. [Department of Physics, University of Kashmir, Srinagar 190 006 (India); Department of Physics and Astronomy, University of Tennessee, Knoxville, TN 37996 (United States); Bhat, G.H. [Department of Physics, University of Kashmir, Srinagar 190 006 (India); Sun, Y., E-mail: sunyang@sjtu.edu.c [Department of Physics, Shanghai Jiao Tong University, Shanghai 200240 (China); Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 730000 (China); Department of Physics and Astronomy, University of Tennessee, Knoxville, TN 37996 (United States); Palit, R. [Department of Nuclear and Atomic Physics, Tata Institute of Fundamental Research, Colaba, Mumbai (India)

    2010-05-10

    Inspired by the recent experimental data [J.-G. Wang, et al., Phys. Lett. B 675 (2009) 420], we extend the triaxial projected shell model approach to study the gamma-band structure in odd-mass nuclei. As a first application of the new development, the gamma-vibrational structure of {sup 103}Nb is investigated. It is demonstrated that the model describes the ground-state band and multi-phonon gamma-vibrations quite satisfactorily, supporting the interpretation of the data as one of the few experimentally-known examples of simultaneous occurrence of one- and two-gamma-phonon vibrational bands. This generalizes the well-known concept of the surface gamma-oscillation in deformed nuclei built on the ground-state in even-even systems to gamma-bands based on quasiparticle configurations in odd-mass systems.

  16. Stellar electron-capture rates in pf-shell nuclei from quasiparticle random-phase approximation calculations

    CERN Document Server

    Sarriguren, P

    2013-01-01

    Electron-capture rates at different density and temperature conditions are evaluated for a set of pf-shell nuclei representative of the constituents in presupernova formations. The nuclear structure part of the problem is described within a quasiparticle random-phase approximation based on a deformed Skyrme Hartree-Fock selfconsistent mean field with pairing correlations and residual interactions in particle-hole and particle-particle channels. The energy distributions of the Gamow-Teller strength are evaluated and compared to benchmark shell-model calculations and experimental data extracted from charge-exchange reactions. The model dependence of the weak rates are discussed and the various sensitivities to both density and temperature are analyzed.

  17. Shell effect and capture cross sections in the synthesis of superheavy nuclei

    Institute of Scientific and Technical Information of China (English)

    DU SaiSai; BIAN BaoAn; LIU Min; FENG ZhaoQing; ZHANG FengShou

    2009-01-01

    The shell effect is included in the improved isospin dependent quantum molecular dynamics model in which the shell correction energy of the system is calculated by using the deformed two-center shell model.A switch function is introduced to connect the shell correction energy of the projectile and the target with that of the compound nucleus during the dynamical fusion process.It is found that the calculated capture cross sections reproduce the experimental data quantitatively at the energy near the Coulomb barrier.The capture cross sections for reaction 8035Br+20882Pb→288117X are also calculated and discussed.

  18. Shell effect and capture cross sections in the synthesis of superheavy nuclei

    Institute of Scientific and Technical Information of China (English)

    2009-01-01

    The shell effect is included in the improved isospin dependent quantum molecular dynamics model in which the shell correction energy of the system is calculated by using the deformed two-center shell model.A switch function is introduced to connect the shell correction energy of the projectile and the target with that of the compound nucleus during the dynamical fusion process.It is found that the calculated capture cross sections reproduce the experimental data quantitatively at the energy near the Coulomb barrier.The capture cross sections for reaction 8305 Br + 28028 Pb → 121878X are also calculated and discussed.

  19. General transformation of α cluster model wave function to jj-coupling shell model in various 4N nuclei

    Science.gov (United States)

    Itagaki, N.; Matsuno, H.; Suhara, T.

    2016-09-01

    The antisymmetrized quasi-cluster model (AQCM) is a method to describe transitions from the α cluster wave functions to jj-coupling shell model wave functions. In this model, the cluster-shell transition is characterized by only two parameters: R representing the distance between α clusters and Λ describing the breaking of α clusters. The contribution of the spin-orbit interaction, very important in the jj-coupling shell model, can be taken into account starting with the α cluster model wave function. In this article we show the generality of AQCM by extending the application to heavier regions: various 4N nuclei from 4He to 100Sn. The characteristic magic numbers of the jj-coupling shell model, 28 and 50, are described starting with the α cluster model. The competition of two different configurations is discussed in 20Ne (16O + one quasi-cluster and 12C + two quasi-clusters) and 28Si (pentagon shape of five quasi-clusters and 12C + 16O). Also, we compare the energy curves for the α + 40Ca cluster configuration calculated with and without the α breaking effect in 44Ti.

  20. Dielectronic recombination measurements of iron M-shell ions motivated by active galactic nuclei X-ray absorption features

    Science.gov (United States)

    Lukic, V. D.; Schnell, M.; Savin, D. W.; Brandau, C.; Schmidt, E. W.; Bohm, S.; Muller, A.; Schippers, S.; Lestinsky, M.; Sprenger, F.; Wolf, A.; Altun, Z.; Badnell, N. R.

    2008-07-01

    XMM-Newton and Chandra observations of active galactic nuclei (AGN) show rich spectra of X-ray absorption lines. These observations have detected a broad unresolved transition array (UTA) between 15-17 A. This is attributed to inner-shell photoexcitation of M-shell iron ions. Modeling these UTA features is currently limited by uncertainties in the low-temperature dielectronic recombination (DR) data for M-shell iron. In order to resolve this issue, and to provide reliable iron M-shell DR data for plasma modeling, we are carrying out a series of laboratory measurements using the heavy-ion Test Storage Ring (TSR) at the Max-Plank-Institute for Nuclear Physics in Heidelberg, Germany. Currently, laboratory measurements of low temperature DR can only be performed at storage rings. We use the DR data obtained at TSR, to calculate rate coefficients for plasma modeling and to benchmark theoretical DR calculations. At temperatures where these ions are predicted to form in photoionized gas, we find a significant discrepancy between our experimental results and previously recommended DR rate coefficients. Here we report our recent experimental results for DR of Mg-like Fe XV forming Al-like Fe XIV.

  1. Investigating neutron-proton pairing in s d -shell nuclei via (p ,3He) and (3He,p ) transfer reactions

    Science.gov (United States)

    Ayyad, Y.; Lee, J.; Tamii, A.; Lay, J. A.; Macchiavelli, A. O.; Aoi, N.; Brown, B. A.; Fujita, H.; Fujita, Y.; Ganioglu, E.; Hatanaka, K.; Hashimoto, T.; Ito, T.; Kawabata, T.; Li, Z.; Liu, H.; Matsubara, H.; Miki, K.; Ong, H. J.; Potel, G.; Sugai, I.; Susoy, G.; Vitturi, A.; Watanabe, H. D.; Yokota, N.; Zenihiro, J.

    2017-08-01

    Neutron-proton pairing correlations are investigated in detail via n p transfer reactions in N =Z s d -shell nuclei. In particular, we study the cross-section ratio of the lowest 0+ and 1+ states as an observable to quantify the interplay between T =0 (isoscalar) and T =1 (isovector) pairing strengths. The experimental results are compared to second-order distorted-wave Born approximation calculations with proton-neutron amplitudes obtained in the shell-model formalism using the universal s d -shell interaction B. Our results suggest underestimation of the nonneglible isoscalar pairing strength in the shell-model descriptions at the expense of the isovector channel.

  2. Manifestation of three-body forces in f7/2-shell nuclei

    CERN Document Server

    Volya, Alexander

    2008-01-01

    The traditional nuclear shell model approach is extended to include many-body forces. The empirical Hamiltonian with a three-body force is constructed for the proton and neutron 0f7/2 shells. Manifestations of the three-body force in spectra, binding energies, seniority mixing, particle-hole symmetry, electromagnetic and particle transition rates are investigated. The model with a three-body force is demonstrated to provide a better agreement with observations as compared to large-scale traditional shell model calculations.

  3. Deformed shell model results for neutrinoless double beta decay of nuclei in A=60-90 region

    CERN Document Server

    Sahu, R

    2014-01-01

    Nuclear transition matrix elements (NTME) for the neutrinoless double beta decay of $^{70}$Zn, $^{80}$Se and $^{82}$Se nuclei are calculated within the framework of the deformed shell model based on Hartree-Fock states. For $^{70}$Zn, jj44b interaction in $^{2}p_{3/2}$, $^{1}f_{5/2}$, $^{2}p_{1/2}$ and $^{1}g_{9/2}$ space with $^{56}$Ni as the core is employed. However, for $^{80}$Se and $^{82}$Se nuclei, a modified Kuo interaction with the above core and model space are employed. Most of our calculations in this region were performed with this effective interaction. However, jj44b interaction has been found to be better for $^{70}$Zn. After ensuring that DSM gives good description of the spectroscopic properties of low-lying levels in these three nuclei considered, the NTME are calculated. The deduced half-lives with these NTME, assuming neutrino mass is 1 eV, are $9.6 \\times 10^{25}$yr, $1.9 \\times 10^{27}$yr and $1.95 \\times 10^{24}$yr for $^{70}$Zn, $^{80}$Se and $^{82}$Se, respectively.

  4. Assessing open-system behavior of 14C in terrestrial gastropod shells

    Science.gov (United States)

    Rech, Jason A.; Pigati, Jeffrey S.; Lehmann, Sophie B.; McGimpsey, Chelsea N.; Grimley, David A.; Nekola, Jeffrey C.

    2011-01-01

    In order to assess open-system behavior of radiocarbon in fossil gastropod shells, we measured the 14C activity on 10 aliquots of shell material recovered from Illinoian (~190-130 ka) and pre-Illinoian (~800 ka) loess and lacustrine deposits in the Midwestern USA. Eight of the 10 aliquots yielded measurable 14C activities that ranged from 0.25 to 0.53 percent modern carbon (pMC), corresponding to apparent 14C ages between 48.2 and 42.1 ka. This small level of open-system behavior is common in many materials that are used for 14C dating (e.g. charcoal), and typically sets the upper practical limit of the technique. Two aliquots of gastropod shells from the Illinoian-aged Petersburg Silt (Petersburg Section) in central Illinois, USA, however, yielded elevated 14C activities of 1.26 and 1.71 pMC, which correspond to apparent 14C ages of 35.1 and 32.7 ka. Together, these results suggest that while many fossil gastropods shells may not suffer from major (>1%) open-system problems, this is not always the case. We then examined the mineralogy, trace element chemistry, and physical characteristics of a suite of fossil and modern gastropod shells to identify the source of contamination in the Petersburg shells and assess the effectiveness of these screening techniques at identifying samples suitable for 14C dating. Mineralogical (XRD) and trace element analyses were inconclusive, which suggests that these techniques are not suitable for assessing open-system behavior in terrestrial gastropod shells. Analysis with scanning electron microscopy (SEM), however, identified secondary mineralization (calcium carbonate) primarily within the inner whorls of the Petersburg shells. This indicates that SEM examination, or possibly standard microscope examination, of the interior of gastropod shells should be used when selecting fossil gastropod shells for 14C dating.

  5. Lifetimes in the middle of 1f{sub 7/2} shell: cross-conjugated nuclei {sup 47}V and {sup 49}Cr

    Energy Technology Data Exchange (ETDEWEB)

    Brandolini, F. E-mail: brandolini@pd.infn.it; Medina, N.H.; Lenzi, S.M.; Napoli, D.R.; Poves, A.; Ribas, R.V.; Sanchez-Solano, J.; Ur, C.A.; De Poli, M.; Marginean, N.; Bazzacco, D.; Cameron, J.A.; De Angelis, G.; Gadea, A.; Menegazzo, R.; Rossi-Alvarez, C

    2001-10-22

    DSAM lifetimes have been determined in the middle of 1f{sub 7/2} shell for the cross-conjugated nuclei {sup 47}V and {sup 49}Cr, populated with the reaction {sup 28}Si on {sup 28}Si at 115 MeV using a Au backed target. B(E2) and B(M1) reduced rates agree very well with large scale shell model predictions. The interplay between spherical and collective structures is discussed.

  6. Diradical character dependences of the first and second hyperpolarizabilities of asymmetric open-shell singlet systems.

    Science.gov (United States)

    Nakano, Masayoshi; Champagne, Benoît

    2013-06-28

    The static first and second hyperpolarizabilities (referred to as β and γ, respectively) of asymmetric open-shell singlet systems have been investigated using the asymmetric two-site diradical model within the valence configuration interaction level of theory in order to reveal the effect of the asymmetric electron distribution on the diradical character and subsequently on β and γ. It is found that the increase of the asymmetric electron distribution causes remarkable changes in the amplitude and the sign of β and γ, and that their variations are intensified with the increase of the diradical character. These results demonstrate that the asymmetric open-shell singlet systems with intermediate diradical characters can exhibit further enhancements of β and γ as compared to conventional asymmetric closed-shell systems and also to symmetric open-shell singlet systems with intermediate diradical characters.

  7. Novel features of nuclear forces and shell evolution in exotic nuclei

    CERN Document Server

    Otsuka, Takaharu; Honma, Michio; Utsuno, Yutaka; Tsunoda, Naofumi; Tsukiyama, Koshiroh; Hjorth-Jensen, Morten

    2009-01-01

    Novel simple properties of the monopole component of the effective nucleon-nucleon interaction are presented, leading to the so-called monopole-based universal interaction. Shell structures are shown to change as functions of $N$ and $Z$ consistently with experiments. Some key cases of this shell evolution are discussed, clarifying the effects of central and tensor forces. The validity of the present tensor force is examined in terms of the low-momentum interaction V$_{low k}$ and the Q$_{box}$ formalism.

  8. Alpha cluster states and molecular orbitals in sd-shell nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Kimura, M. [Creative Research Institution Sousei Research Department, Hokkaido University, Sapporo 001-0021 (Japan); Furutachi, N. [Meme Media Laboratory, Hokkaido University, Sapporo 060-8628 (Japan); Kanada-En' yo, Y. [Yukawa Institute for Theoretical Physics, Kyoto University, Kyoto 606-8502 (Japan)

    2010-03-01

    The alpha-clustering and molecular-orbitals of {sup 22}Ne and F isotopes are investigated based on antisymmetrized molecular dynamics (AMD). The observed candidates for the alpha cluster state of {sup 22}Ne are understood as the molecular-orbital states and alpha+{sup 18}O di-nuclei states. The presence of the molecular-orbital states in the O and F isotopes and the drastic reduction of their excitation energy near the neutron-drip line are predicted.

  9. Free vibration analysis of open circular cylindrical shells by the method of reverberation-ray matrix

    Directory of Open Access Journals (Sweden)

    Dong Tang

    2016-03-01

    Full Text Available This article is concerned with free vibration analysis of open circular cylindrical shells with either the two straight edges or the two curved edges simply supported and the remaining two edges supported by arbitrary classical boundary conditions. An analytical solution of the traveling wave form along the simply supported edges and the standing wave form along the remaining two edges is obtained based on the Flügge thin shell theory. With such a unidirectional traveling wave form solution, the method of reverberation-ray matrix is introduced to derive the equation of natural frequencies of the open circular cylindrical shell with various boundary conditions. Then, the golden section search algorithm is employed to obtain the natural frequencies of the open circular cylindrical shell. The calculation results are compared with those obtained by the finite element method and the method in available literature. Finally, the natural frequencies of the open circular cylindrical shell with various boundary conditions are calculated and the effects of boundary conditions on the natural frequencies are examined. The calculation results can be used as benchmark values for researchers to check their numerical methods and for engineers to design thin structures with shell components.

  10. Beta-decay of nuclei around Se-90. Search for signatures of a N=56 sub-shell closure relevant the r-process

    CERN Document Server

    Quinn, M; Pereira, J; Surman, R; Arndt, O; Baumann, T; Becerril, A; Elliot, T; Estrade, A; Galaviz, D; Ginter, T; Hausmann, M; Hennrich, S; Kessler, R; Kratz, K -L; Lorusso, G; Mantica, P F; Matos, M; Moller, P; Montes, F; Pfeiffer, B; Portillo, M; Hennrich, S; Schatz, H; Schertz, F; Schnorrenberger, L; Smith, E; Stolz, A; Walters, W B; Wohr, A

    2011-01-01

    Nuclear structure plays a significant role on the rapid neutron capture process (r-process) since shapes evolve with the emergence of shells and sub-shells. There was some indication in neighboring nuclei that we might find examples of a new N=56 sub-shell, which may give rise to a doubly magic Se-90 nucleus. Beta-decay half lives of nuclei around Se-90 have been measured to determine if this nucleus has in fact a doubly-magic character. The fragmentation of Xe-136 beam at the National Superconducting Cyclotron Laboratory at Michigan State University was used to create a cocktail of nuclei in the A=90 region. We have measured the half lives of twenty-two nuclei near the r-process path in the A=90 region. The half lives of As-88 and Se-90 have been measured for the first time. The values were compared with theoretical predictions in the search for nuclear-deformation signatures of a N=56 sub-shell, and its possible role in the emergence of a potential doubly-magic Se-90. The impact of such hypothesis on the sy...

  11. Electromagnetic properties in {sup 160-170}Dy nuclei. A microscopic description by the pseudo-SU(3) shell model

    Energy Technology Data Exchange (ETDEWEB)

    Vargas, Carlos E.; Bagatella-Flores, Norma [Universidad Veracruzana, Facultad de Fisica, Veracruz (Mexico); Velazquez, Victor [Universidad Nacional Autonoma de Mexico, Facultad de Ciencias, Mexico D.F. (Mexico); Lerma-Hernandez, Sergio [Universidad Veracruzana, Facultad de Fisica, Veracruz (Mexico); Universidad Nacional Autonoma de Mexico, Instituto de Ciencias Nucleares, Mexico D.F. (Mexico)

    2017-04-15

    The large collectivity observed in the rare-earth region of the nuclear landscape is well known. The microscopic studies are difficult to perform in this region due to the enormous size of the valence spaces, a problem that can be avoided by means of the use of symmetry-based models. Here we present calculations for electromagnetic properties of {sup 160-170}Dy nuclei within the pseudo-SU(3) scheme. The model Hamiltonian includes the preserving symmetry Q.Q term and the symmetry-breaking Nilsson and pairing terms, systematically parametrized for all members of the chain. The model is used to calculate B(E2) and B(M1) inter-band transition strengths between the ground state, γ and β-bands. In addition, we present results for quadrupole moments and g factors in these rotational bands. The results show that the pseudo-SU(3) shell model is a powerful microscopic theory for a description of electromagnetic properties of states in the normal parity sector in heavy deformed nuclei. (orig.)

  12. Understanding emergent collectivity and clustering in nuclei from a symmetry-based no-core shell-model perspective

    CERN Document Server

    Dreyfuss, A C; Dytrych, T; Draayer, J P; Baker, R B; Deibel, C M; Bahri, C

    2016-01-01

    We present a detailed discussion of the structure of the low-lying positive-parity energy spectrum of $^{12}$C from a no-core shell-model perspective. The approach utilizes a fraction of the usual shell-model space and extends its multi-shell reach via the symmetry-based no-core symplectic shell model (NCSpM) with a simple, physically-informed effective interaction. We focus on the ground-state rotational band, the Hoyle state and its $2^+$ and $4^+$ excitations, as well as the giant monopole $0^+$ resonance, which is a vibrational breathing mode of the ground state. This, in turn, allows us to address the open question about the structure of the Hoyle state and its rotational band. In particular, we find that the Hoyle state is best described through deformed prolate collective modes rather than vibrational modes, while we show that the higher-lying giant monopole $0^+$ resonance resembles the oblate deformation of the $^{12}$C ground state. In addition, we identify the giant monopole $0^+$ and quadrupole $2...

  13. Formation of Hyper Hydrogen isotopes in light p-shell nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Jolos, R. V., E-mail: jolos@theor.jinr.ru [JINR, Bogoliubov Laboratory of Theoretical Physics (Russian Federation); Majling, L. [Nuclear Physics Institute (Czech Republic); Majlingova, O. [Czech Technical University (Czech Republic)

    2016-11-15

    Recent experiment by A1 Collaboration at Mainz, namely identification of {sub Λ}{sup 4}H hyperfragment from primary {sub Λ}{sup 9}Li hypernucleus produced in reaction (e, e′K{sup +}), stirred renewed interest in baryonic decay of hypernuclei. The important role of s{sup −1}s{sub Λ} excitation in p-shell hypernuclei as well as the existence of selection rules connected with [f] (Young diagram) was noted earlier within Translational Invariant Shell Model (TISM). The particular conditions of the present experiment (reaction is not selective and produces highly excited states) dictate extension of the simplest TISM: expansion of the harmonic oscillator basis space and compression of multiplets (to only (λμ) for L and [f] for S, T). Such modified TISM explains abundance production of {sub Λ}{sup 4}H hyperfragment and predicts production of another Hyper Hydrogen {sub Λ}{sup 6}H.

  14. Shell model estimate of electric dipole moments in medium and heavy nuclei

    Science.gov (United States)

    Teruya, E.; Yoshinaga, N.; Higashiyama, K.

    2014-03-01

    It is evidence for an extension of the Standard Model in particle physics, if static electric dipole moments (EDMs) are measured for any elementary particle. The nuclear EDM arises mainly from two sources: one comes from asymmetric charge distribution in a nucleus and the other is due to the nucleon intrinsic EDM. We estimate the nuclear EDMs from two sources for the 1/21+ states in Xe isotopes by a shell model approach using full orbitals between magic numbers 50 and 82.

  15. Deformed shell model study of heavy N=Z nuclei and dark matter detection

    CERN Document Server

    Sahu, R

    2016-01-01

    Deformed shell model (DSM) based on Hartree-Fock intrinsic states is applied to address two current problems of interest. Firstly, in the $f_{5/2}pg_{9/2}$ model space with jj44b effective interaction along with isospin projection, DSM is used to describe the structure of the recently observed low-lying $T=0$ and $T=1$ bands in the heavy odd-odd N=Z nucleus $^{66}$As. DSM results are close to the data and also to the shell model results. For the $T=1$ band, DSM predicts structural change at $8^+$ just as in the shell model. In addition, the lowest two $T=0$ bands are found to have quasi-deuteron structure above a $^{64}$Ge core and the $5^+$ and $9^+$ levels of the third $T=0$ band are found to be isomeric states. Secondly, in a first application of DSM to dark matter, detection rates for the lightest supersymmetric particle (a dark matter candidate) are calculated with $^{73}$Ge as the detector.

  16. Kinetically blocked stable heptazethrene and octazethrene: Closed-shell or open-shell in the ground state?

    KAUST Repository

    Li, Yuan

    2012-09-12

    Polycyclic aromatic hydrocarbons with an open-shell singlet biradical ground state are of fundamental interest and have potential applications in materials science. However, the inherent high reactivity makes their synthesis and characterization very challenging. In this work, a convenient synthetic route was developed to synthesize two kinetically blocked heptazethrene (HZ-TIPS) and octazethrene (OZ-TIPS) compounds with good stability. Their ground-state electronic structures were systematically investigated by a combination of different experimental methods, including steady-state and transient absorption spectroscopy, variable temperature NMR, electron spin resonance (ESR), superconducting quantum interfering device (SQUID), FT Raman, and X-ray crystallographic analysis, assisted by unrestricted symmetry-broken density functional theory (DFT) calculations. All these demonstrated that the heptazethrene derivative HZ-TIPS has a closed-shell ground state while its octazethrene analogue OZ-TIPS with a smaller energy gap exists as an open-shell singlet biradical with a large measured biradical character (y = 0.56). Large two-photon absorption (TPA) cross sections (σ(2)) were determined for HZ-TIPS (σ(2)max = 920 GM at 1250 nm) and OZ-TIPS (σ(2)max = 1200 GM at 1250 nm). In addition, HZ-TIPS and OZ-TIPS show a closely stacked 1D polymer chain in single crystals. © 2012 American Chemical Society.

  17. Shell model estimate of electric dipole moments in medium and heavy nuclei

    Science.gov (United States)

    Teruya, Eri; Yoshinaga, Naotaka; Higashiyama, Koji

    2015-05-01

    Existence of the electric dipole moment (EDM) is deeply related with time-reversal invariance. The EDMof a diamagnetic atom is mainly induced by the nuclear Schiff moment. After carrying out the shell model calculations to obtain wavefunctions for Xe isotopes, we evaluate nuclear Schiff moments for Xe isotopes to estimate their atomic EDMs. We estimate the contribution from each single particle orbital for the Schiff moment. It is found that the contribution on the Schiff moment is very different from orbital to orbital.

  18. Shell model estimate of electric dipole moments in medium and heavy nuclei

    Directory of Open Access Journals (Sweden)

    Teruya Eri

    2015-01-01

    Full Text Available Existence of the electric dipole moment (EDM is deeply related with time-reversal invariance. The EDMof a diamagnetic atom is mainly induced by the nuclear Schiff moment. After carrying out the shell model calculations to obtain wavefunctions for Xe isotopes, we evaluate nuclear Schiff moments for Xe isotopes to estimate their atomic EDMs. We estimate the contribution from each single particle orbital for the Schiff moment. It is found that the contribution on the Schiff moment is very different from orbital to orbital.

  19. Shell model estimate of electric dipole moments in medium and heavy nuclei

    Directory of Open Access Journals (Sweden)

    Teruya E.

    2014-03-01

    Full Text Available It is evidence for an extension of the Standard Model in particle physics, if static electric dipole moments (EDMs are measured for any elementary particle. The nuclear EDM arises mainly from two sources: one comes from asymmetric charge distribution in a nucleus and the other is due to the nucleon intrinsic EDM. We estimate the nuclear EDMs from two sources for the 1/21+ states in Xe isotopes by a shell model approach using full orbitals between magic numbers 50 and 82.

  20. Superheavy nuclei

    CERN Document Server

    Sáro, S

    2003-01-01

    Experiments leading to transuranium and far transuranium nuclei as far as element 106 (seaborgium) are described. Physical knowledge derived from experimental data at this stage of complete synthesis nuclear reactions since the 1980s is analyzed. The effect of the shell structure on the stability of the nuclei, the extra-push effect, and the effect of isospin are discussed. Experiments leading to the synthesis of nuclei with Z = 107 - 112 by cold fusion are also described, as are hot fusion reactions resulting in superheavy nuclei Z = 114, 116 where, however, confirmation is only pending. Current state of the art in this area is also highlighted

  1. Electromagnetic properties of neutron-rich nuclei adjacent to the Z=50 shell closure

    Directory of Open Access Journals (Sweden)

    M. Rejmund

    2016-02-01

    Full Text Available Low-lying high-spin yrast states in the exotic odd–odd isotopes 124–128Sb (Z=51 and 118–128In (Z=49, studied for the first time, show a striking difference in their observed γ-ray decay. With a single valence proton particle/hole occupying the g7/2/g9/2 spin-orbit partners, dominant electric quadrupole transitions occur in Sb as opposed to magnetic dipole transitions in In. The observed properties are explained on the basis of general principles of symmetry and with large-scale shell-model calculations, and reveal novel aspects of the competition between the neutron–proton interaction and the like-nucleon pairing interaction.

  2. Low Energy Positive-Negative Pion Interactions with S-D Shell Nuclei.

    Science.gov (United States)

    Tacik, Roman

    A magnetic spectrometer has been commissioned for use in performing low energy pion scattering experiments. It has been used to measure the differential cross sections for the elastic scattering of 50 MeV (pi)('(+OR-)) from ('12)C, ('18)O, and ('26)Mg targets, as well as the inelastic scattering to the 2(,1)('+) states of these nuclei. The analysis of the elastic scattering data has been performed with an optical potential model. It is found that the (pi)('(+OR-)) elastic cross sections for ('12)C and ('18)O are well described by calculations employ - ing a global parameter set('1), which has been previously shown to reproduce (pi)('(+OR-)) elastic scattering data for a range of nuclei. The (pi)('(+OR-)) elastic data for ('26)Mg require a variation of the p-wave potential parameters. A similar requirement is seen with (pi)('(+OR -)) - ('32)S elastic data('2). Distorted wave calculations, inputting separate neutron and pro- ton transition densities, have been performed for the analysis of the inelastic data. These calculations demonstrate a strong sensitivity of (pi)('(+OR-)) to protons, and (pi)('-) to neutrons, present in the nucleus. By varying the strengths of the neutron and proton transition densities, in order to reproduce the (pi)('(+OR -)) inelastic cross sections, it is possible to determine the ratio of neutron to proton matrix elements (M(,n)/M(,p)) for the given 2('+) states. It is shown that the value of M(,n)/M(,p) obtained in this way is independent of the optical potential param- eters used in the calculation. The extracted values of M(,n)/M(,p) are: 0.97 (+OR-) 0.08, 1.81 (+OR-) 0.15, and 0.90 (+OR-) 0.07 for ('12)C, ('18)O, and ('26)Mg. respectively. These values are in agreement with those obtained by other means. ('1)J. A. Carr et. al., Phys Rev C25 (82) 952. ('2)R. J. Sobie, PhD Thesis, University of Toronto, 1984.

  3. The {\\it ab initio} calculation of spectra of open shell diatomic molecules

    CERN Document Server

    Tennyson, Jonathan; McKemmish, Laura K; Yurchenko, Sergei N

    2016-01-01

    The spectra (rotational, rotation-vibrational or electronic) of diatomic molecules due to transitions involving only closed-shell ($^1\\Sigma$) electronic states follow very regular, simple patterns and their theoretical analysis is usually straightforward. On the other hand, open-shell electronic states lead to more complicated spectral patterns and, moreover, often appear as a manifold of closely lying electronic states, leading to perturbations with even larger complexity. This is especially true when at least one of the atoms is a transition metal. Traditionally these complex cases have been analysed using approaches based on perturbation theory, with semi-empirical parameters determined by fitting to spectral data. Recently the needs of two rather diverse scientific areas have driven the demand for improved theoretical models of open-shell diatomic systems based on an \\emph{ab initio} approach, these areas are ultracold chemistry and the astrophysics of "cool" stars, brown dwarfs and most recently extraso...

  4. Alpha-decay of deformed superheavy nuclei as a probe of shell closures

    Science.gov (United States)

    Ismail, M.; Seif, W. M.; Adel, A.; Abdurrahman, A.

    2017-02-01

    A systematic study on α-decay half-life time, Tα, of α-particle emission from a large number of deformed heavy and superheavy nuclei is presented. The calculations are employed in the framework of the density-dependent cluster model. The microscopic α-daughter nuclear interaction potential is calculated in the framework of the double-folding model with the realistic effective Michigan-three-Yukawa Reid nucleon-nucleon interaction. We study the neutron number variation of log Tα and arranged different isotones at each neutron magic number according to their stability, in the sense that the more stable isotone corresponds to the lowest value of log Tα. We found that the half-life time becomes minimum when the neutron or proton numbers of the corresponding daughter nucleus are magic. Moreover, the half-life time is maximum for parent nucleus with magicity. The nuclear stability is assumed to be proportional with the depth of the minimum value in log Tα for the daughter nucleus or the height of its maximum value for the parent one. The neutron magic numbers predicted and confirmed from the present study are 126, 152, 162, 172, 184, 196, 202 and 212, most of them were deduced by other authors based on different methods.

  5. Mechanism of Rh-Catalyzed Oxidative Cyclizations: Closed versus Open Shell Pathways.

    Science.gov (United States)

    Park, Yoonsu; Ahn, Seihwan; Kang, Dahye; Baik, Mu-Hyun

    2016-06-21

    A conceptual theory for analyzing and understanding oxidative addition reactions that form the cornerstone of many transition metal mediated catalytic cycles that activate C-C and C-H bonds, for example, was developed. The cleavage of the σ- or π-bond in the organic substrate can be envisioned to follow a closed or an open shell formalism, which is matched by a corresponding electronic structure at the metal center of the catalyst. Whereas the assignment of one or the other mechanistic scenario appears formal and equivalent at first sight, they should be recognized as different classes of reactions, because they lead to different reaction optimization and control strategies. The closed-shell mechanism involves heterolytic bond cleavages, which give rise to highly localized charges to form at the transition state. In the open-shell pathway, bonds are broken homolytically avoiding localized charges to accumulate on molecular fragments at the transition states. As a result, functional groups with inductive effects may exert a substantial influence on the energies of the intermediate and transition states, whereas no such effect is expected if the mechanism proceeds through the open-shell mechanism. If these functional groups are placed in a way that opens an electronic communication pathway to the molecular sites where charges accumulate, for example, using hyperconjugation, electron donating groups may stabilize a positive charge at that site. An instructive example is discussed, where this stereoelectronic effect allowed for rendering the oxidative addition diastereoselective. No such control is possible, however, when the open-shell reaction pathway is followed, because the inductive effects of functional groups have little to no effect on the stabilities of radical-like substrate states that are encountered when the bonds are broken in a homolytic fashion. Whether the closed-shell or open-shell mechanism for oxidative addition is followed is determined by the

  6. Charge-changing transitions and capture strengths of pf-shell nuclei with $T_{z} = -2$ at proton drip-line

    CERN Document Server

    Rahman, Muneeb-Ur

    2016-01-01

    Charge-changing transitions, commonly referred to as Gamow-Teller (GT) transitions, and electron capture/$\\beta^{+}$-decay strengths for pf-shell nuclei with $T_{z} = - 2$ at proton drip-line have been calculated using the proton-neutron quasi-particle random phase approximation (pn-QRPA) model. The total GT$_{+}$ strength values and electron capture/$\\beta^{+}$-decay rates are needed for the study of the late stages of the stellar evolution. The pn-QRPA theory is used for a microscopic calculation of GT strength distribution functions and associated stellar electron capture/$\\beta^{+}$-decay rates of proton-rich pf-shell nuclei with $T_{z} = - 2$ in the mass range 46 $\\leq$ A $\\leq$ 56 at proton drip-line. Standard quenching factor of 0.74, usually implemented in the shell model calculation, has been incorporated for the comparison with experimental data (wherever available). The calculated GT strength of the two proton-rich nuclei, $^{52}$Ni and $^{56}$Zn are compared with experimental data of corresponding...

  7. Half-life systematics across the N=126 shell closure: role of first-forbidden transitions in the β decay of heavy neutron-rich nuclei.

    Science.gov (United States)

    Morales, A I; Benlliure, J; Kurtukián-Nieto, T; Schmidt, K-H; Verma, S; Regan, P H; Podolyák, Z; Górska, M; Pietri, S; Kumar, R; Casarejos, E; Al-Dahan, N; Algora, A; Alkhomashi, N; Álvarez-Pol, H; Benzoni, G; Blazhev, A; Boutachkov, P; Bruce, A M; Cáceres, L S; Cullen, I J; Denis Bacelar, A M; Doornenbal, P; Estévez-Aguado, M E; Farrelly, G; Fujita, Y; Garnsworthy, A B; Gelletly, W; Gerl, J; Grebosz, J; Hoischen, R; Kojouharov, I; Kurz, N; Lalkovski, S; Liu, Z; Mihai, C; Molina, F; Mücher, D; Rubio, B; Shaffner, H; Steer, S J; Tamii, A; Tashenov, S; Valiente-Dobón, J J; Walker, P M; Wollersheim, H J; Woods, P J

    2014-07-11

    This Letter reports on a systematic study of β-decay half-lives of neutron-rich nuclei around doubly magic (208)Pb. The lifetimes of the 126-neutron shell isotone (204)Pt and the neighboring (200-202)Ir, (203)Pt, (204)Au are presented together with other 19 half-lives measured during the "stopped beam" campaign of the rare isotope investigations at GSI collaboration. The results constrain the main nuclear theories used in calculations of r-process nucleosynthesis. Predictions based on a statistical macroscopic description of the first-forbidden β strength reveal significant deviations for most of the nuclei with Nforbidden transitions reproduce more satisfactorily the trend in the measured half-lives for the nuclei in this region, where the r-process pathway passes through during β decay back to stability.

  8. The single-nucleon energies of closed shell nuclei, influenced by n(k,rho), in the framework of Hartree-Fock inspired-scheme and LOCV method

    CERN Document Server

    Mariji, Hodjat

    2016-01-01

    The nucleon single-particle energies (SPEs) of the selected closed shell nuclei; that is, 16O, 40Ca, and 56Ni, are obtained by using the diagonal matrix elements of two-body effective interaction, which generated through the lowest order constrained variational (LOCV) calculations for the symmetric nuclear matter with the AV18 phenomenological nucleon-nucleon potential. The SPEs at the major levels of nuclei are calculated by employing a Hartree-Fock inspired-scheme in the spherical harmonic oscillator basis. In the scheme, the correlation influences are taken into account by imposing the nucleon effective mass factor on the radial wave functions of the major levels. Replacing the density-dependent one-body momentum distribution functions of nucleons, n(k,rho), with the Heaviside functions, the role of n(k,rho) on the nucleon SPEs at the major levels of the selected closed shell nuclei, is investigated. The best fit of spin-orbit splitting is taken into account when correcting the major levels of the nuclei b...

  9. Three-body forces and persistence of spin-orbit shell gaps in medium-mass nuclei: Toward the doubly magic 78Ni

    Science.gov (United States)

    Sieja, K.; Nowacki, F.

    2012-05-01

    We present state-of-the-art shell-model calculations in a large model space (pf for protons, fpgd for neutrons), which allows us to study simultaneously excitations across the Z=28 and N=50 shell gaps. We explore the region in the vicinity of 78Ni, which is a subject of intense experimental investigations. Our calculations correctly account for the known low-lying excited states in this region, including those which may correspond to cross-shell excitations. We observe the minimum of the N=50 mass gap at Z=32 consistent with experimental data and its further increase toward Z=28, indicating a robustness of the N=50 gap in 78Ni. The evolution of the N=50 gap along the nickel chain is shown to bear similarities to what is known in oxygen and calcium chains, providing a new opportunity for the studies of three-body monopole effects in medium-mass nuclei.

  10. Rate coefficients of open shell molecules and radicals: $R$-matrix method

    Indian Academy of Sciences (India)

    JASMEET SINGH; K L BALUJA; GAGANDEEP LONGIANY

    2017-05-01

    The open shell molecules with even number of electrons have $\\pi^2$ or $\\pi^{2}_{g}$ ground-state electronic configuration. Several homonuclear diatomic molecules like $\\rm{O_2, S_2, B_2}$ have $\\pi^{2}_{g}$ ground state in the $D_{\\infty h}$ point group and heteronuclear diatomic radicals like PH, NH, SO have $\\pi^2$ ground state in the $C_{\\infty v}$ point group. We have computed and presented here the rate coefficient of these open shell molecules $\\rm{(O_2, S_2, B_2)}$ and radicals (PH, NH,SO) from the results of our previous studies using a well-established $\\it {ab-initio}$ formalism: the $R$-matrix method. The rate coefficients for elastic and electron-excited processes are studied over a wide electron temperature range.

  11. Description of nuclear systems with a self-consistent configuration-mixing approach. II: Application to structure and reactions in even-even sd-shell nuclei

    CERN Document Server

    Robin, C; Dupuis, M; Bloas, J Le; Arteaga, D Peña; Berger, J -F

    2016-01-01

    The variational multiparticle-multihole configuration mixing approach (MPMH) to nuclei has been proposed about a decade ago. While the first applications followed rapidly, the implementation of the full formalism of this method has only been recently completed and applied in [C. Robin, N. Pillet, D. Pe\\~na Arteaga and J.-F. Berger, Phys. Rev. C 93, 024302 (2016)] to $^{12}$C as a test-case. The main objective of the present paper is to carry on the study that was initiated in that reference, in order to put the MPMH method to more stringent tests. To that aim we perform a systematic study of even-even sd-shell nuclei. The wave function of these nuclei is taken as a configuration mixing built on orbitals of the sd-shell, and both the mixing coefficients of the nuclear state and the single-particle wave functions are determined consistently from the same variational principle. The calculations are done using the D1S Gogny force. Various ground-state properties are analyzed. In particular, the correlation conten...

  12. The ab initio calculation of spectra of open shell diatomic molecules

    Science.gov (United States)

    Tennyson, Jonathan; Lodi, Lorenzo; McKemmish, Laura K.; Yurchenko, Sergei N.

    2016-05-01

    The spectra (rotational, rotation-vibrational or electronic) of diatomic molecules due to transitions involving only closed-shell (1Σ ) electronic states follow very regular, simple patterns and their theoretical analysis is usually straightforward. On the other hand, open-shell electronic states lead to more complicated spectral patterns and, moreover, often appear as a manifold of closely lying electronic states, leading to perturbed spectra of even greater complexity. This is especially true when at least one of the atoms is a transition metal. Traditionally these complex cases have been analysed using approaches based on perturbation theory, with semi-empirical parameters determined by fitting to spectral data. Recently the needs of two rather diverse scientific areas have driven the demand for improved theoretical models of open-shell diatomic systems based on an ab initio approach; these areas are ultracold chemistry and the astrophysics of ‘cool’ stars, brown dwarfs and most recently extrasolar planets. However, the complex electronic structure of these molecules combined with the accuracy requirements of high-resolution spectroscopy render such an approach particularly challenging. This review describes recent progress in developing methods for directly solving the effective Schrödinger equation for open-shell diatomic molecules, with a focus on molecules containing a transtion metal. It considers four aspects of the problem: (i) the electronic structure problem; (ii) non-perturbative treatments of the curve couplings; (iii) the solution of the nuclear motion Schrödinger equation; (iv) the generation of accurate electric dipole transition intensities. Examples of applications are used to illustrate these issues.

  13. Excited states of large open-shell molecules: an efficient, general, and spin-adapted approach based on a restricted open-shell ground state wave function.

    Science.gov (United States)

    Roemelt, Michael; Neese, Frank

    2013-04-11

    A spin-adapted configuration interaction with singles method that is based on a restricted open-shell reference function (ROCIS) with general total spin S is presented. All excited configuration state functions (CSFs) are generated with the aid of a spin-free second quantization formalism that only leads to CSFs within the first order interacting space. By virtue of the CSF construction, the formalism involves higher than singly excited determinants but not higher than singly excited configurations. Matrix elements between CSFs are evaluated on the basis of commutator relationships using a symbolic algebra program. The final equations were, however, hand-coded in order to maximize performance. The method can be applied to fairly large systems with more than 100 atoms in reasonable wall-clock times and also parallelizes well. Test calculations demonstrate that the approach is far superior to UHF-based configuration interaction with single excitations but necessarily falls somewhat short of quantitative accuracy due to the lack of dynamic correlation contributions. In order to implicitly account for dynamic correlation in a crude way, the program optionally allows for the use of Kohn-Sham orbitals in combination with a modest downscaling of two-electron integrals (DFT/ROCIS). All two-electron integrals of Kohn-Sham orbitals that appear in the Hamiltonian matrix are reduced by a total of three scaling parameters that are suitable for a wide range of molecules. Test calculations on open-shell organic radicals as well as transition metal complexes demonstrate the wide applicability of the method and its ability to calculate the electronic spectra of large molecular systems.

  14. Generalized Møller-Plesset Multiconfiguration Perturbation Theory Applied to an Open-Shell Antisymmetric Product of Strongly Orthogonal Geminals Reference Wave Function.

    Science.gov (United States)

    Tarumi, Moto; Kobayashi, Masato; Nakai, Hiromi

    2012-11-13

    The antisymmetric product of strongly orthogonal geminals (APSG) method is a wave function theory that can effectively treat the static electron correlation. Recently, we proposed the open-shell APSG method using one-electron orbitals for open-shell parts. In this paper, we have extended the perturbation correction to the open-shell APSG calculations through Møller-Plesset-type multiconfiguration perturbation theory (MP-MCPT). Numerical applications demonstrate that the present open-shell MP-MCPT can reasonably reproduce the dissociation energies or equilibrium distances for open-shell systems.

  15. Decamethylytterbocene Complexes of Bipyridines and Diazabutadienes: Multiconfigurational Ground States and Open-Shell Singlet Formation

    Energy Technology Data Exchange (ETDEWEB)

    Booth, Corwin H.; Walter, Marc D.; Kazhdan, Daniel; Hu, Yung-Jin; Lukens, Wayne W.; Bauer, Eric D.; Maron, Laurent; Eisenstein, Odile; Andersen, Richard A.

    2009-04-22

    Partial ytterbium f-orbital occupancy (i.e., intermediate valence) and open-shell singlet formation are established for a variety of bipyridine and diazabutadiene adducts with decamethylytterbocene, (C5Me5)2Yb, abbreviated as Cp*2Yb. Data used to support this claim include ytterbium valence measurements using Yb LIII-edge X-ray absorption near-edge structure spectroscopy, magnetic susceptibility, and complete active space self-consistent field (CASSCF) multiconfigurational calculations, as well as structural measurements compared to density functional theory calculations. The CASSCF calculations indicate that the intermediate valence is the result of a multiconfigurational ground-state wave function that has both an open-shell singlet f13(?*)1, where pi* is the lowest unoccupied molecular orbital of the bipyridine or dpiazabutadiene ligands, and a closed-shell singlet f14 component. A number of other competing theories for the unusual magnetism in these materials are ruled out by the lack of temperature dependence of the measured intermediate valence. These results have implications for understanding chemical bonding not only in organolanthanide complexes but also for f-element chemistry in general, as well as understanding magnetic interactions in nanoparticles and devices.

  16. Decamethylytterbocene complexes of bipyridines and diazabutadines: multiconfigurational ground states and open-shell singlet formation

    Energy Technology Data Exchange (ETDEWEB)

    Bauer, Eric D [Los Alamos National Laboratory; Booth, C H [LBNL; Walter, M D [LBNL; Kazhdan, D [LBNL; Hu, Y - J [LBNL; Lukens, Wayne [LBNL; Maron, Laurent [INSA TOULOUSE; Eisentein, Odile [UNIV MONTPELLIER 2; Anderson, Richard [LBNL

    2009-01-01

    Partial ytterbium f-orbital occupancy (i.e. intermediate valence) and open-shell singlet Draft 12/formation are established for a variety of bipyridine and diazabutadiene adducts to decamethylytterbocene, (C{sub 5}Me{sub 5}){sub 2}Yb or Cp*{sub 2}Yb. Data used to support this claim includes ytterbium valence measurements using Yb Lm-edge x-ray absorption near-edge structure (XANES) spectroscopy, magnetic susceptibility and Complete Active Space Self-Consistent Field (CASSCF) multi configurational calculations, as well as structural measurements compared to density-functional theory (DFT) calculations. The CASSCF calculations indicate that the intermediate valence is the result of a multiconfigurational ground state wave function that has both an open-shell singlet f{sup 13} and a closed-shell singlet f{sup 14} component. A number of other competing theories for the unusual magnetism in these materials are ruled out by the presence of intermediate valence and its lack of any significant temperature dependence. These results have implications for understanding chemical bonding not only in organolanthanide complexes, but also for organometallic chemistry in general, as well as understanding magnetic interactions in nanopartic1es and devices.

  17. Investigation of the structure of core-coupled odd-proton copper nuclei in fpg valence space using the projected shell model

    Energy Technology Data Exchange (ETDEWEB)

    Gupta, Anuradha; Singh, Suram; Bharti, Arun [University of Jammu, Department of Physics and Electronics, Jammu (India); Khosa, S.K. [Central University of Jammu, Department of Physics and Astronomical Sciences, Jammu (India); Bhat, G.H.; Sheikh, J.A. [University of Kashmir, Department of Physics, Srinagar (India)

    2017-01-15

    By employing a systematically parametrized Hamiltonian and the best fit of the various input parameters, high-spin yrast energy states for an isotopic chain of odd mass {sup 59-69}Cu nuclei have been investigated by using a novel computational quantum mechanical framework-projected shell model. Comparison of calculations and experiments yields good agreement. The present study of various intriguing nuclear structure properties along the yrast lines in these odd proton isotopes reflects some interesting informative nuclear physics results. The calculations successfully describe the formation of the yrast level structures from multi-quasi-particle configurations based on πf x νg bands for {sup 59-69}Cu isotopes. The present calculations indicate the evolution of the nuclear structure near the magic nuclei, Ni, and also provide an indication of coexistence of both, collective as well as single-particle, levels for {sup 69}Cu nucleus at N=40. (orig.)

  18. Open structure ZnO/CdSe core/shell nanoneedle arrays for solar cells.

    Science.gov (United States)

    Chen, Yanxue; Wei, Lin; Zhang, Guanghua; Jiao, Jun

    2012-09-20

    Open structure ZnO/CdSe core/shell nanoneedle arrays were prepared on a conducting glass (SnO2:F) substrate by solution deposition and electrochemical techniques. A uniform CdSe shell layer with a grain size of approximately several tens of nanometers was formed on the surface of ZnO nanoneedle cores after annealing at 400°C for 1.5 h. Fabricated solar cells based on these nanostructures exhibited a high short-circuit current density of about 10.5 mA/cm2 and an overall power conversion efficiency of 1.07% with solar illumination of 100 mW/cm2. Incident photo-to-current conversion efficiencies higher than 75% were also obtained.

  19. Measurements of gamma rays from keV-neutron resonance capture by odd-Z nuclei in the 2s-1d shell region

    Energy Technology Data Exchange (ETDEWEB)

    Igashira, Masayuki; Lee, Sam Yol; Mizuno, Satoshi; Hori, Jun-ichi [Tokyo Inst. of Tech. (Japan). Research Lab. for Nuclear Reactors; Kitazawa, Hideo

    1998-03-01

    Measurements of gamma rays from keV-neutron resonance capture by {sup 19}F, {sup 23}Na, and {sup 27}Al, which are odd-Z nuclei in the 2s-1d shell region, were performed, using an anti-Compton HPGe spectrometer and a pulsed neutron source by the {sup 7}Li(p,n){sup 7}Be reaction. Capture gamma rays from the 27-, 49-, and 97-keV resonances of {sup 19}F, the 35- and 53-keV resonances of {sup 23}Na, and the 35-keV resonance of {sup 27}Al were observed. Some results are presented. (author)

  20. Description of nuclear systems with a self-consistent configuration-mixing approach. II. Application to structure and reactions in even-even s d -shell nuclei

    Science.gov (United States)

    Robin, C.; Pillet, N.; Dupuis, M.; Le Bloas, J.; Peña Arteaga, D.; Berger, J.-F.

    2017-04-01

    Background: The variational multiparticle-multihole configuration mixing approach to nuclei has been proposed about a decade ago. While the first applications followed rapidly, the implementation of the full formalism of this method has only been recently completed and applied in C. Robin, N. Pillet, D. Peña Arteaga, and J.-F. Berger, [Phys. Rev. C 93, 024302 (2016)], 10.1103/PhysRevC.93.024302 to 12C as a test-case. Purpose: The main objective of the present paper is to carry on the study that was initiated in that reference, in order to put the variational multiparticle-multihole configuration mixing method to more stringent tests. To that aim we perform a systematic study of even-even s d -shell nuclei. Method: The wave function of these nuclei is taken as a configuration mixing built on orbitals of the s d -shell, and both the mixing coefficients of the nuclear state and the single-particle wave functions are determined consistently from the same variational principle. As in the previous works, the calculations are done using the D1S Gogny force. Results: Various ground-state properties are analyzed. In particular, the correlation content and composition of the wave function as well as the single-particle orbitals and energies are examined. Binding energies and charge radii are also calculated and compared to experiment. The description of the first excited state is also examined and the corresponding transition densities are used as input for the calculation of reaction processes such as inelastic electron and proton scattering. Special attention is paid to the effect of the optimization of the single-particle states consistently with the correlations of the system. Conclusions: The variational multiparticle-multihole configuration mixing approach is systematically applied to the description of even-even s d -shell nuclei. Globally, the results are satisfying and encouraging. In particular, charge radii and excitation energies are nicely reproduced. However

  1. Stability analysis of an open shallow cylindrical shell with imperfection under external pressure

    Directory of Open Access Journals (Sweden)

    Psotny Martin

    2017-01-01

    Full Text Available Elastic shallow generalized cylindrical shells of an open cross-section subjected to the various forms of external pressure are analysed in the paper numerically using the finite element method. Load - displacement paths are calculated for the perfect and imperfect geometry, respectively. Special attention is paid to the influence of initial geometric imperfection on the limit load level of fundamental equilibrium path of nonlinear analysis. ANSYS system was used for analysis, arc-length method was chosen for obtaining fundamental load - displacement path of solution.

  2. Pathological behavior of the open-shell restricted self-consistent-field equations

    Energy Technology Data Exchange (ETDEWEB)

    Moscardo, F.; Alvarez-Collado, J.R.

    1979-02-01

    The possible solutions of open-shell restricted self-consistent-field equations for a doublet are studied for Li and Na atoms, according to the values of the parameters implied in those equations. A similar behavior, characterized by the presence of several variational solutions is observed in both atoms. Some of these solutions can be assigned to excited configurations. Excitation energies are in good agreement with experimental data. Doublet stability for the solutions obtained has been studied, discussing the saddle-point character present in those solutions associated to excited configurations.

  3. Remnants of spherical shell structures in deformed nuclei: The impact of an N=64 neutron subshell closure on the structure of N~90 gadolinium nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Ross, T.J. [University of Richmond; Hughes, R.O. [University of Richmond; Beausang, C.W. [University of Richmond; Allmond, James M [ORNL; Angell, C.T. [Lawrence Berkeley National Laboratory (LBNL); Basunia, M.S. [Lawrence Berkeley National Laboratory (LBNL); Bleuel, D.L. [Lawrence Livermore National Laboratory (LLNL); Burke, J.T. [Lawrence Livermore National Laboratory (LLNL); Casperson, R.J. [Lawrence Livermore National Laboratory (LLNL); Escher, J.E. [Lawrence Livermore National Laboratory (LLNL); Fallon, P. [Lawrence Berkeley National Laboratory (LBNL); Hatarik, R. [Lawrence Berkeley National Laboratory (LBNL); Munson, J. [Lawrence Berkeley National Laboratory (LBNL); Paschalis, S. [Lawrence Berkeley National Laboratory (LBNL); Petri, M. [Lawrence Berkeley National Laboratory (LBNL); Phair, L. [Lawrence Berkeley National Laboratory (LBNL); Ressler, J.J. [Lawrence Livermore National Laboratory (LLNL); Scielzo, N.D. [Lawrence Livermore National Laboratory (LLNL)

    2013-01-01

    Odd-mass gadolinium isotopes around N = 90 were populated by the (p,d ) reaction, utilizing 25-MeV protons, resulting in population of low-spin quasineutron states at energies near and below the Fermi surface. Systematics of the single quasineutron levels populated are presented. A large excitation energy gap is observed between levels originating from the 2d3/2 , 1h11/2 , and 3s1/2 spherical parents (above the N = 64 gap), and the 2d5/2 (below the gap), indicating that the spherical shell model level spacing is maintained at least to moderate deformations.

  4. Shell

    OpenAIRE

    Harper, Catherine

    2006-01-01

    Susie MacMurray's Shell installation manifests in Pallant House Gallery, Chichester, like some pulsing exotica, a heavily-textured wall-paper, darkly decorative, heavily luxurious, broodingly present, with more than a hint of the uncanny or the gothic. A remarkable undertaking by an artist of significance, this work's life-span will be just one year, and then it will disappear, leaving no physical trace, but undoubtedly contributing in a much less tangible way to an already rich layering of n...

  5. Coulomb excitation of neutron-rich nuclei between the N=40 and N=50 shell gaps using REX-ISOLDE and the Ge MINIBALL array

    CERN Multimedia

    2002-01-01

    We propose to perform Coulomb excitation experiments of neutron-rich nuclei in the vicinity of $^{68}$Ni towards $^{78}$Ni using the REX-ISOLDE facility coupled with the highly efficient MINIBALL array. Major changes in the structure of the atomic nucleus are expected around the N = 40 subshell closure. Recent B(E2) measurements suggested that $^{68}$Ni behaves like a doubly magic nucleus while neutron-rich Zn isotopes with N>38 exhibit a sudden increase of B(E2) values which may be the signature of deformation. We would like to check and test these predictions for neutron-rich nuclei in the vicinity of N = 40 and N = 50 shell closures like $^{72}$Zn, $^{74}$Zn, $^{76}$Zn, $^{68}$Ni, $^{70}$Ni. Our calculations show that an energy upgrade from 2.2 to 3 MeV/nucleon will be of crucial importance for a part of our study while some nuclei can still be very efficiently studied at an energy of 2.2 MeV/nucleon. Therefore, to perform our experiment in an efficient way, we request 21 shifts of beam time before the ene...

  6. Stable tetrabenzo-Chichibabin's hydrocarbons: Tunable ground state and unusual transition between their closed-shell and open-shell resonance forms

    KAUST Repository

    Zeng, Zebing

    2012-09-05

    Stable open-shell polycyclic aromatic hydrocarbons (PAHs) are of fundamental interest due to their unique electronic, optical, and magnetic properties and promising applications in materials sciences. Chichibabin\\'s hydrocarbon as a classical open-shell PAH has been investigated for a long time. However, most of the studies are complicated by their inherent high reactivity. In this work, two new stable benzannulated Chichibabin\\'s hydrocarbons 1-CS and 2-OS were prepared, and their electronic structure and geometry in the ground state were studied by various experiments (steady-state and transient absorption spectra, NMR, electron spin resonance (ESR), superconducting quantum interference device (SQUID), FT Raman, X-ray crystallographic etc.) and density function theory (DFT) calculations. 1-CS and 2-OS exhibited tunable ground states, with a closed-shell quinoidal structure for 1-CS and an open-shell biradical form for 2-OS. Their corresponding excited-state forms 1-OS and 2-CS were also chemically approached and showed different decay processes. The biradical 1-OS displayed an unusually slow decay to the ground state (1-CS) due to a large energy barrier (95 ± 2.5 kJ/mol) arising from severe steric hindrance during the transition from an orthogonal biradical form to a butterfly-like quinoidal form. The quick transition from the quinoidal 2-CS (excited state) to the orthogonal biradicaloid 2-OS (ground state) happened during the attempted synthesis of 2-CS. Compounds 1-CS and 2-OS can be oxidized into stable dications by FeCl 3 and/or concentrated H 2SO 4. The open-shell 2-OS also exhibited a large two-photon absorption (TPA) cross section (760 GM at 1200 nm). © 2012 American Chemical Society.

  7. Symmetry-adapted perturbation theory utilizing density functional description of monomers for high-spin open-shell complexes.

    Science.gov (United States)

    Zuchowski, Piotr S; Podeszwa, Rafał; Moszyński, Robert; Jeziorski, Bogumił; Szalewicz, Krzysztof

    2008-08-28

    We present an implementation of symmetry-adapted perturbation theory (SAPT) to interactions of high-spin open-shell monomers forming high-spin dimers. The monomer spin-orbitals used in the expressions for the electrostatic and exchange contributions to the interaction energy are obtained from density functional theory using a spin-restricted formulation of the open-shell Kohn-Sham (ROKS) method. The dispersion and induction energies are expressed through the density-density response functions predicted by the time-dependent ROKS theory. The method was applied to several systems: NH...He, CN...Ne, H2O...HO2, and NH...NH. It provides accuracy comparable to that of the best previously available methods such as the open-shell coupled-cluster method with single, double, and noniterative triple excitations, RCCSD(T), with a significantly reduced computational cost.

  8. Time-dependent density functional methods for Raman spectra in open-shell systems.

    Science.gov (United States)

    Aquino, Fredy W; Schatz, George C

    2014-01-16

    We present an implementation of a time-dependent density functional theory (TD-DFT) linear response module in NWChem for unrestricted DFT calculations and apply it to the calculation of resonant Raman spectra in open-shell molecular systems using the short-time approximation. The new source code was validated and applied to simulate Raman spectra on several doublet organic radicals (e.g., benzyl, benzosemiquinone, TMPD, trans-stilbene anion and cation, and methyl viologen) and the metal complex copper phthalocyanine. We also introduce a divide-and-conquer approach for the evaluation of polarizabilities in relatively large systems (e.g., copper phthalocyanine). The implemented tool gives comparisons with experiment that are similar to what is commonly found for closed-shell systems, with good agreement for most features except for small frequency shifts, and occasionally large deviations for some modes that depend on the molecular system studied, experimental conditions not being accounted in the modeling such as solvation effects and extra solvent-based peaks, and approximations in the underlying theory. The approximations used in the quantum chemical modeling include (i) choice of exchange-correlation functional and basis set; (ii) harmonic approximation used in the frequency analysis to determine vibrational normal modes; and (iii) short-time approximation (omission of nuclear motion effects) used in calculating resonant Raman spectra.

  9. Predicted Landé g-factors for open shell diatomic molecules

    Science.gov (United States)

    Semenov, Mikhail; Yurchenko, Sergei. N.; Tennyson, Jonathan

    2016-12-01

    The program DUO (Yurchenko et al., 2016) provides direct solutions of the nuclear motion Schrödinger equation for the (coupled) potential energy curves of open shell diatomic molecules. Wavefunctions from DUO are used to compute Landé g-factors valid for weak magnetic fields; the results are compared with the idealized predictions of both Hund's case (a) and Hund's case (b) coupling schemes. Test calculations are performed for AlO, NO, CrH and C2. The computed gJ 's both provide a sensitive test of the underlying spectroscopic model used to represent the system and an indication of whether states of the molecule are well-represented by the either of the Hund's cases considered. The computation of Landé g-factors is implemented as a standard option in the latest release of DUO.

  10. Infrared-dressed entanglement of cold open-shell polar molecules for universal matchgate quantum computing

    CERN Document Server

    Herrera, Felipe; Kais, Sabre; Whaley, K Birgitta

    2014-01-01

    Implementing a scalable quantum information processor using polar molecules in optical lattices requires precise control over the long-range dipole-dipole interaction between molecules in selected lattice sites. We present here a scheme using trapped open-shell $^2\\Sigma$ polar molecules that allows dipolar exchange processes between nearest and next-nearest neighbors to be controlled to construct a generalized transverse Ising spin Hamiltonian with tunable $XX$, $YY$ and $XY$ couplings in the rotating frame of the driving lasers. The scheme requires a moderately strong bias magnetic field with near-infrared light to provide local tuning of the qubit energy gap, and mid-infrared pulses to perform rotational state transfer via stimulated Raman adiabatic passage. No interaction between qubits is present in the absence of the infrared driving. We analyze the fidelity of the resulting two-qubit matchgate, and demonstrate its robustness as a function of the driving parameters. We discuss a realistic application of...

  11. Shell-model description of the non-compound component of nucleon induced reactions on light and medium nuclei for nucleon incident energies up to 12 MeV

    CERN Document Server

    Orlin, V N

    2002-01-01

    A coupled-channels approach in intermediate coupling shell model for describing the non-compound component of nucleon-nucleus reactions is proposed. The goal of the model is to take into account the influence of collective doorway states (giant resonances) on the characteristics of nucleon-induced reactions on light and medium nuclei for incident energies epsilon <= 12 MeV

  12. Endohedral metallofullerenes, M@C60 (M = Ca, Na, Sr): selective adsorption and sensing of open-shell NOx gases.

    Science.gov (United States)

    Tawfik, Sherif Abdulkader; Cui, X Y; Ringer, S P; Stampfl, C

    2016-08-21

    Based on density-functional theory and non-equilibrium Green's function calculations, we demonstrate that endohedral metallofullerenes (EMFs) are reactive to open-shell gases, and therefore have the potential application as selective open-shell gas sensors. The adsorption of eight gas species (CO, H2O, H2S, NO2, NO, SO2, O2 and NH3) on three EMFs (M@C60, M = Ca, Na and Sr) shows that the adsorption energies of the EMFs towards NO2 and NO are significantly higher than the closed-shell species. Moreover, the high selectivity appears relatively insensitive to the inserted metal atoms. The calculated current-voltage characteristics of gold-M@C60-gold structures (M = Ca, Na) show that the adsorption of NO2 leads to significant change in conductivity, suggesting a potential application as an EMF gas resistive sensing device.

  13. Spin-adapted open-shell time-dependent density functional theory. II. Theory and pilot application.

    Science.gov (United States)

    Li, Zhendong; Liu, Wenjian; Zhang, Yong; Suo, Bingbing

    2011-04-07

    The excited states of open-shell systems calculated by unrestricted Kohn-Sham-based time-dependent density functional theory (U-TD-DFT) are often heavily spin-contaminated and hence meaningless. This is solved ultimately by the recently proposed spin-adapted time-dependent density functional theory (TD-DFT) (S-TD-DFT) [J. Chem. Phys. 133, 064106 (2010)]. Unlike the standard restricted open-shell Kohn-Sham-based TD-DFT (R-TD-DFT) which can only access the singlet-coupled single excitations, the S-TD-DFT can capture both the singlet- and triplet-coupled single excitations with the same computational effort as the U-TD-DFT. The performances of the three approaches (U-TD-DFT, R-TD-DFT, and S-TD-DFT) are compared for both the spin-conserving and spin-flip excitations of prototypical open-shell systems, the nitrogen (N(2)(+)) and naphthalene (C(10)H(8)(+)) cations. The results show that the S-TD-DFT gives rise to balanced descriptions of excited states of open-shell systems.

  14. Open-shell pair interaction energy decomposition analysis (PIEDA): formulation and application to the hydrogen abstraction in tripeptides.

    Science.gov (United States)

    Green, Mandy C; Fedorov, Dmitri G; Kitaura, Kazuo; Francisco, Joseph S; Slipchenko, Lyudmila V

    2013-02-21

    An open-shell extension of the pair interaction energy decomposition analysis (PIEDA) within the framework of the fragment molecular orbital (FMO) method is developed. The open-shell PIEDA method allows the analysis of inter- and intramolecular interactions in terms of electrostatic, exchange-repulsion, charge-transfer, dispersion, and optional polarization energies for molecular systems with a radical or high-spin fragment. Taking into account the low computational cost and scalability of the FMO and PIEDA methods, the new scheme provides a means to characterize the stabilization of radical and open-shell sites in biologically relevant species. The open-shell PIEDA is applied to the characterization of intramolecular interactions in capped trialanine upon hydrogen abstraction (HA) at various sites on the peptide. Hydrogen abstraction reaction is the first step in the oxidative pathway initiated by reactive oxygen or nitrogen species, associated with oxidative stress. It is found that HA results in significant geometrical reorganization of the trialanine peptide. Depending on the HA site, terminal interactions in the radical fold conformers may become weaker or stronger compared to the parent molecule, and often change the character of the non-covalent bonding from amide stacking to hydrogen bonding.

  15. Super-Radiant Dynamics, Doorways, and Resonances in Nuclei and Other Open Mesoscopic Systems

    CERN Document Server

    Auerbach, Naftali

    2011-01-01

    The phenomenon of super-radiance (Dicke effect, coherent spontaneous radiation by a gas of atoms coupled through the common radiation field) is well known in quantum optics. The review discusses similar physics that emerges in open and marginally stable quantum many-body systems. In the presence of open decay channels, the intrinsic states are coupled through the continuum. At sufficiently strong continuum coupling, the spectrum of resonances undergoes the restructuring with segregation of very broad super-radiant states and trapping of remaining long-lived compound states. The appropriate formalism describing this phenomenon is based on the Feshbach projection method and effective non-Hermitian Hamiltonian. A broader generalization is related to the idea of doorway states connecting quantum states of different structure. The method is explained in detail and the examples of applications are given to nuclear, atomic and particle physics. The interrelation of the collective dynamics through continuum and possi...

  16. Assessment of the accuracy of coupled cluster perturbation theory for open-shell systems. I. Triples expansions.

    Science.gov (United States)

    Eriksen, Janus J; Matthews, Devin A; Jørgensen, Poul; Gauss, Jürgen

    2016-05-21

    The accuracy at which total energies of open-shell atoms and organic radicals may be calculated is assessed for selected coupled cluster perturbative triples expansions, all of which augment the coupled cluster singles and doubles (CCSD) energy by a non-iterative correction for the effect of triple excitations. Namely, the second- through sixth-order models of the recently proposed CCSD(T-n) triples series [J. J. Eriksen et al., J. Chem. Phys. 140, 064108 (2014)] are compared to the acclaimed CCSD(T) model for both unrestricted as well as restricted open-shell Hartree-Fock (UHF/ROHF) reference determinants. By comparing UHF- and ROHF-based statistical results for a test set of 18 modest-sized open-shell species with comparable RHF-based results, no behavioral differences are observed for the higher-order models of the CCSD(T-n) series in their correlated descriptions of closed- and open-shell species. In particular, we find that the convergence rate throughout the series towards the coupled cluster singles, doubles, and triples (CCSDT) solution is identical for the two cases. For the CCSD(T) model, on the other hand, not only its numerical consistency, but also its established, yet fortuitous cancellation of errors breaks down in the transition from closed- to open-shell systems. The higher-order CCSD(T-n) models (orders n > 3) thus offer a consistent and significant improvement in accuracy relative to CCSDT over the CCSD(T) model, equally for RHF, UHF, and ROHF reference determinants, albeit at an increased computational cost.

  17. Critical Assessment of TD-DFT for Excited States of Open-Shell Systems: I. Doublet-Doublet Transitions.

    Science.gov (United States)

    Li, Zhendong; Liu, Wenjian

    2016-01-12

    A benchmark set of 11 small radicals is set up to assess the performance of time-dependent density functional theory (TD-DFT) for the excited states of open-shell systems. Both the unrestricted (U-TD-DFT) and spin-adapted (X-TD-DFT) formulations of TD-DFT are considered. For comparison, the well-established EOM-CCSD (equation-of-motion coupled-cluster with singles and doubles) is also used. In total, 111 low-lying singly excited doublet states are accessed by all the three approaches. Taking the MRCISD+Q (multireference configuration interaction with singles and doubles plus the Davidson correction) results as the benchmark, it is found that both U-TD-DFT and EOM-CCSD perform well for those states dominated by singlet-coupled single excitations (SCSE) from closed-shell to open-shell, open-shell to vacant-shell, or closed-shell to vacant-shell orbitals. However, for those states dominated by triplet-coupled single excitations (TCSE) from closed-shell to vacant-shell orbitals, both U-TD-DFT and EOM-CCSD fail miserably due to severe spin contaminations. In contrast, X-TD-DFT provides balanced descriptions of both SCSE and TCSE. As far as the functional dependence is concerned, it is found that, when the Hartree-Fock ground state does not suffer from the instability problem, both global hybrid (GH) and range-separated hybrid (RSH) functionals perform grossly better than pure density functionals, especially for Rydberg and charge-transfer excitations. However, if the Hartree-Fock ground state is instable or nearly instable, GH and RSH tend to underestimate severely the excitation energies. The SAOP (statistically averaging of model orbital potentials) performs more uniformly than any other density functionals, although it generally overestimates the excitation energies of valence excitations. Not surprisingly, both EOM-CCSD and adiabatic TD-DFT are incapable of describing excited states with substantial double excitation characters.

  18. Assessment of the accuracy of coupled cluster perturbation theory for open-shell systems. I. Triples expansions

    CERN Document Server

    Eriksen, Janus Juul; Jørgensen, Poul; Gauss, Jürgen

    2015-01-01

    The accuracy with which total energies of open-shell species may be calculated using coupled cluster perturbative triples expansions is investigated. In particular, the acclaimed CCSD(T) model, in which a non-iterative correction for the effect of triple excitations is added to the coupled cluster singles and doubles (CCSD) energy, is compared to the second- through sixth-order models of the recently proposed CCSD(T-n) triples series for both unrestricted as well as restricted open-shell Hartree-Fock (UHF/ROHF) reference determinants. By comparing UHF- and ROHF-based statistical results for a test set of 18 atoms and small radicals with comparable RHF-based results, it is found that not only the numerical consistency of the CCSD(T) model, but also its fortuitous cancellation of errors for closed-shell systems break down in the transition from closed- to open-shell systems. For the higher-order models of the CCSD(T-n) series, however, no behavioral differences are found between the correlated descriptions of c...

  19. Realistic calculations for c coefficients of the isobaric mass multiplet equation in 1 p 0 f shell nuclei

    Science.gov (United States)

    Ormand, W. E.; Brown, B. A.; Hjorth-Jensen, M.

    2017-08-01

    We present calculations for the c coefficients of the isobaric mass multiplet equation for nuclei from A =42 to A =54 based on input from three realistic nucleon-nucleon interactions. We demonstrate that there is a clear dependence on the short-range charge-symmetry-breaking (CSB) part of the strong interaction and that there is significant disagreement in the CSB part between the commonly used CD-Bonn, chiral effective field theory at next-to-next-to-next-to-leading-order, and Argonne V18 nucleon-nucleon interactions. In addition, we show that all three interactions give a CSB contribution to the c coefficient that is too large when compared to experiment.

  20. Hydration Gibbs free energies of open and closed shell trivalent lanthanide and actinide cations from polarizable molecular dynamics.

    Science.gov (United States)

    Marjolin, Aude; Gourlaouen, Christophe; Clavaguéra, Carine; Ren, Pengyu Y; Piquemal, Jean-Philip; Dognon, Jean-Pierre

    2014-10-01

    The hydration free energies, structures, and dynamics of open- and closed-shell trivalent lanthanide and actinide metal cations are studied using molecular dynamics simulations (MD) based on a polarizable force field. Parameters for the metal cations are derived from an ab initio bottom-up strategy. MD simulations of six cations solvated in bulk water are subsequently performed with the AMOEBA polarizable force field. The calculated first-and second shell hydration numbers, water residence times, and free energies of hydration are consistent with experimental/theoretical values leading to a predictive modeling of f-elements compounds.

  1. Spin-adapted open-shell time-dependent density functional theory. III. An even better and simpler formulation.

    Science.gov (United States)

    Li, Zhendong; Liu, Wenjian

    2011-11-21

    The recently proposed spin-adapted time-dependent density functional theory (S-TD-DFT) [Z. Li and W. Liu, J. Chem. Phys. 133, 064106 (2010)] resolves the spin-contamination problem in describing singly excited states of high spin open-shell systems. It is an extension of the standard restricted open-shell Kohn-Sham-based TD-DFT which can only access those excited states due to singlet-coupled single excitations. It is also far superior over the unrestricted Kohn-Sham-based TD-DFT (U-TD-DFT) which suffers from severe spin contamination for those excited states due to triplet-coupled single excitations. Nonetheless, the accuracy of S-TD-DFT for high spin open-shell systems is still inferior to TD-DFT for well-behaved closed-shell systems. The reason can be traced back to the violation of the spin degeneracy conditions (SDC) by approximate exchange-correlation (XC) functionals. Noticing that spin-adapted random phase approximation (S-RPA) can indeed maintain the SDC by virtue of the Wigner-Eckart theorem, a hybrid ansatz combining the good of S-TD-DFT and S-RPA can immediately be envisaged. The resulting formalism, dubbed as X-TD-DFT, is free of spin contamination and can also be viewed as a S-RPA correction to the XC kernel of U-TD-DFT. Compared with S-TD-DFT, X-TD-DFT leads to much improved results for the low-lying excited states of, e.g., N(2)(+), yet with much reduced computational cost. Therefore, X-TD-DFT can be recommended for routine calculations of excited states of high spin open-shell systems.

  2. Relativistic equation-of-motion coupled-cluster method using open-shell reference wavefunction

    CERN Document Server

    Pathak, Himadri; Nayak, Malaya K; Vaval, Nayana; Pal, Sourav

    2016-01-01

    The open-shell reference relativistic equation-of-motion coupled-cluster method within its four-component description is successfully implemented with the consideration of single- and double- excitation approximation. The one-body and two-body matrix elements required for the correlation calculation are generated using Dirac-Coulomb Hamiltonian. As a first attempt, the implemented method is employed to calculate a few of the low-lying ionized states of heavy atomic (Ag, Cs, Au, Fr, Lr) and valence ionization potential of molecular (HgH, PbF) systems, where the effect of relativity does really matter to obtain highly accurate results. Not only the relativistic effect, but also the effect of electron correlation is crucial in these heavy atomic and molecular systems. To justify the fact, we have taken two further approximations in the four-component relativistic equation-of-motion framework to quantify how the effect of electron correlation plays a role in the calculated values at different level of the approxi...

  3. Time-dependent density functional theory for nonlinear properties of open-shell systems.

    Science.gov (United States)

    Rinkevicius, Zilvinas; Jha, Prakash Chandra; Oprea, Corneliu I; Vahtras, Olav; Agren, Hans

    2007-09-21

    This paper presents response theory based on a spin-restricted Kohn-Sham formalism for computation of time-dependent and time-independent nonlinear properties of molecules with a high spin ground state. The developed approach is capable to handle arbitrary perturbations and constitutes an efficient procedure for evaluation of electric, magnetic, and mixed properties. Apart from presenting the derivation of the proposed approach, we show results from illustrating calculations of static and dynamic hyperpolarizabilities of small Si(3n+1)H(6n+3) (n=0,1,2) clusters which mimic Si(111) surfaces with dangling bond defects. The results indicate that the first hyperpolarizability tensor components of Si(3n+1)H(6n+3) have an ordering compatible with the measurements of second harmonic generation in SiO2/Si(111) interfaces and, therefore, support the hypothesis that silicon surface defects with dangling bonds are responsible for this phenomenon. The results exhibit a strong dependence on the quality of basis set and exchange-correlation functional, showing that an appropriate set of diffuse functions is required for reliable predictions of the first hyperpolarizability of open-shell compounds.

  4. Allowance for the shell structure of the {sub 42}{sup 100}Mo and {sub 46}{sup 110}Pd nuclei in the synthesis of {sub 84}{sup 200}Po, {sub 88}{sup 210}Ra, and {sub 92}{sup 220}U

    Energy Technology Data Exchange (ETDEWEB)

    Litnevsky, V. L., E-mail: vlad.lit@bk.ru [Joint Institute for Nuclear Research, Laboratory of Theoretical Physics (Russian Federation); Kosenko, G. I., E-mail: kosenko@phys.omsu.omskreg.ru [Omsk State University (Russian Federation); Ivanyuk, F. A., E-mail: ivanyuk@voliacable.com [National Academy of Sciences of Ukraine, Institute of Nuclear Research (Ukraine); Pashkevich, V. V., E-mail: pashkevi@theor.jinr.ru [Joint Institute for Nuclear Research, Laboratory of Theoretical Physics (Russian Federation)

    2012-01-15

    The effect of the shell structure of colliding nuclei in calculating the entrance channel on the ensuing evolution of the product system is investigated. The entrance channel is calculated under the assumption of the nose-to-nose orientation of colliding nuclei. The following three reactions involving nuclei that are deformed in the ground state are considered: {sub 42}{sup 100}Mo + {sub 42}{sup 100}Mo {yields} {sub 84}{sup 100}Po, {sub 42}{sup 100}Mo + {sub 46}{sup 100}Pd {yields} {sub 88}{sup 210}Ra, and {sub 46}{sup 110}Pd + {sub 46}{sup 110}Pd {yields} {sub 92}{sup 220}U. The state of the system at the point of touching is determined by the results obtained by calculating the entrance reaction channel. The shape of the system is specified by three collective coordinates (deformation parameters). The evolution of collective coordinates of the system is described in terms of Langevin equations. The potential energy of the system of colliding nuclei is calculated with allowance for their shell structure. It is shown that allowance for individual features of interacting nuclei in the entrance channel of the fusion-fission reactions makes it possible to obtain, for the reactions being considered, cross sections for evaporation-residue formation that are closer to available experimental data than their liquid-drop counterparts.

  5. Toward the Ab-initio Description of Medium Mass Nuclei

    CERN Document Server

    Barbieri, C; Soma, V; Duguet, T; Navratil, P

    2012-01-01

    As ab-initio calculations of atomic nuclei enter the A=40-100 mass range, a great challenge is how to approach the vast majority of open-shell (degenerate) isotopes. We add realistic three-nucleon interactions to the state of the art many-body Green's function theory of closed-shells, and find that physics of neutron driplines is reproduced with very good quality. Further, we introduce the Gorkov formalism to extend ab-initio theory to semi-magic, fully open-shell, isotopes. Proof-of-principle calculations for Ca-44 and Ni-74 confirm that this approach is indeed feasible. Combining these two advances (open-shells and three-nucleon interactions) requires longer, technical, work but it is otherwise within reach.

  6. Efficient and accurate local single reference correlation methods for high-spin open-shell molecules using pair natural orbitals

    Science.gov (United States)

    Hansen, Andreas; Liakos, Dimitrios G.; Neese, Frank

    2011-12-01

    A production level implementation of the high-spin open-shell (spin unrestricted) single reference coupled pair, quadratic configuration interaction and coupled cluster methods with up to doubly excited determinants in the framework of the local pair natural orbital (LPNO) concept is reported. This work is an extension of the closed-shell LPNO methods developed earlier [F. Neese, F. Wennmohs, and A. Hansen, J. Chem. Phys. 130, 114108 (2009), 10.1063/1.3086717; F. Neese, A. Hansen, and D. G. Liakos, J. Chem. Phys. 131, 064103 (2009), 10.1063/1.3173827]. The internal space is spanned by localized orbitals, while the external space for each electron pair is represented by a truncated PNO expansion. The laborious integral transformation associated with the large number of PNOs becomes feasible through the extensive use of density fitting (resolution of the identity (RI)) techniques. Technical complications arising for the open-shell case and the use of quasi-restricted orbitals for the construction of the reference determinant are discussed in detail. As in the closed-shell case, only three cutoff parameters control the average number of PNOs per electron pair, the size of the significant pair list, and the number of contributing auxiliary basis functions per PNO. The chosen threshold default values ensure robustness and the results of the parent canonical methods are reproduced to high accuracy. Comprehensive numerical tests on absolute and relative energies as well as timings consistently show that the outstanding performance of the LPNO methods carries over to the open-shell case with minor modifications. Finally, hyperfine couplings calculated with the variational LPNO-CEPA/1 method, for which a well-defined expectation value type density exists, indicate the great potential of the LPNO approach for the efficient calculation of molecular properties.

  7. Detecting, sourcing, and age-dating dredged sediments on the open shelf, southern California, using dead mollusk shells.

    Science.gov (United States)

    Bizjack, Matthew T; Kidwell, Susan M; Velarde, Ronald G; Leonard-Pingel, Jill; Tomašových, Adam

    2017-01-15

    Molluscan shell debris is an under-exploited means of detecting, sourcing, and age-dating dredged sediments in open-shelf settings. Backscatter features on the Southern California shelf are suggestive of dredged sediment hauled from San Diego Bay but deposited significantly inshore of the EPA-designated ocean disposal site. We find that 36% of all identifiable bivalve shells >2mm (44% of shells >4mm) in sediment samples from this 'short dump' area are from species known to live exclusively in the Bay; such shells are absent at reference sites of comparable water depth, indicating that their presence in the short-dump area signals non-compliant disposal rather than natural offshore transport or sea level rise. These sediments lack the shells of species that invaded California bays in the 1970s, suggesting that disposal preceded federal regulations. This inexpensive, low-tech method, with its protocol for rejecting alternative hypotheses, will be easy to adapt in other settings. Copyright © 2016 Elsevier Ltd. All rights reserved.

  8. Communication: Spin densities within a unitary group based spin-adapted open-shell coupled-cluster theory: Analytic evaluation of isotropic hyperfine-coupling constants for the combinatoric open-shell coupled-cluster scheme

    Energy Technology Data Exchange (ETDEWEB)

    Datta, Dipayan, E-mail: datta.dipayan@gmail.com; Gauss, Jürgen, E-mail: gauss@uni-mainz.de [Institut für Physikalische Chemie, Johannes Gutenberg-Universität Mainz, Duesbergweg 10-14, D-55128 Mainz (Germany)

    2015-07-07

    We report analytical calculations of isotropic hyperfine-coupling constants in radicals using a spin-adapted open-shell coupled-cluster theory, namely, the unitary group based combinatoric open-shell coupled-cluster (COSCC) approach within the singles and doubles approximation. A scheme for the evaluation of the one-particle spin-density matrix required in these calculations is outlined within the spin-free formulation of the COSCC approach. In this scheme, the one-particle spin-density matrix for an open-shell state with spin S and M{sub S} = + S is expressed in terms of the one- and two-particle spin-free (charge) density matrices obtained from the Lagrangian formulation that is used for calculating the analytic first derivatives of the energy. Benchmark calculations are presented for NO, NCO, CH{sub 2}CN, and two conjugated π-radicals, viz., allyl and 1-pyrrolyl in order to demonstrate the performance of the proposed scheme.

  9. Second-order Møller-Plesset perturbation theory without basis set superposition error. II. Open-shell systems.

    Science.gov (United States)

    Salvador, P; Mayer, I

    2004-04-01

    The basis set superposition error-free second-order Møller-Plesset perturbation theory of intermolecular interactions, based on the "chemical Hamiltonian approach," which has been introduced in Part I, is applied here to open-shell systems by using a new, effective computer realization. The results of the numerical examples considered (CH(4) em leader HO, NO em leader HF) showed again the perfect performance of the method. Striking agreement has again been found with the results of the a posteriori counterpoise correction (CP) scheme in the case of large, well-balanced basis sets, which is also in agreement with a most recent formal theoretical analysis. The difficulties of the CP correction in open-shell systems are also discussed.

  10. Carbon-Carbon Bond Formation in a Weak Ligand Field: Leveraging Open Shell First Row Transition Metal Catalysts.

    Science.gov (United States)

    Chirik, Paul James

    2017-01-12

    Unique features of Earth abundant transition metal catalysts are reviewed in the context of catalytic carbon-carbon bond forming reactions. Aryl-substituted bis(imino)pyridine iron and cobalt dihalide compounds, when activated with alkyl aluminum reagents, form highly active catalysts for the polymerization of ethylene. Open shell iron and cobalt alkyl complexes have been synthesized that serve as single component olefin polymerization catalysts. Reduced bis(imino)pyridine iron- and cobalt dinitrogen compounds have also been discovered that promote the unique [2+2] cycloaddition of unactivated terminal alkenes. Electronic structure studies support open shell intermediates, a deviation from traditional strong field organometallic compounds that promote catalytic C-C bond formation.

  11. Systematic study of favored \\alpha-decay half-lives of closed shell odd-A and doubly-odd nuclei related to ground and isomeric states

    CERN Document Server

    Sun, Xiao-Dong; Li, Xiao-Hua

    2016-01-01

    In this work, we systematically investigate the favored $\\alpha$-decay half-lives and $\\alpha$ preformation probabilities of both odd-$A$ and doubly-odd nuclei related to ground and isomeric states around the doubly magic cores at $Z=82$, $N=82$ and at $Z=82$, $N=126$, respectively, within a two-potential approach from the view of the valence nucleon (or hole). The results show that the $\\alpha$ preformation probability is linear related to $N_\\text{p}N_\\text{n}$ or $N_\\text{p}N_\\text{n}I$, where $N_\\text{p}$, $N_\\text{n}$, and $I$ are the number of valence protons (or holes), the number of valence neutrons (or holes), and the isospin of the parent nucleus, respectively. Fitting the $\\alpha$ preformation probabilities data extracted from the differences between experimental data and calculated half-lives without a shell correction, we give two analytic formulas of the $\\alpha$ preformation probabilities and the values of corresponding parameters. Using those formulas and the parameters, we calculate the $\\alp...

  12. Configuration interaction effect on open M shell Fe and Ni LTE spectral opacities, Rosseland and Planck means

    Science.gov (United States)

    Gilles, D.; Busquet, M.; Gilleron, F.; Klapisch, M.; Pain, J.-C.

    2016-05-01

    We have recently shown that iron and nickel open M-shell opacity spectra, up to Δn = 2 are very sensitive to Configuration Interaction (CI) treatments at temperature around 15 eV and for various densities. To do so we had compared extensive CI calculations obtained with two opacity codes HULLAC-v9 and SCO-RCG. In this work we extend these comparisons to a first evaluation of CI effects on Rosseland and Planck means.

  13. Restricted open-shell Kohn-Sham theory for π-π* transitions. I. Polyenes, cyanines, and protonated imines

    Science.gov (United States)

    Grimm, Stephan; Nonnenberg, Christel; Frank, Irmgard

    2003-12-01

    We present a self-consistent field algorithm for the restricted open-shell Kohn-Sham method which can be used to calculate excited states that have the same spatial symmetry as the corresponding ground states. The method is applied to π-π* transitions in polyenes, cyanines, and protonated imines. Excitation energies obtained with gradient corrected functionals are found to be significantly redshifted; the shift is constant within a homologous series. Planar excited state geometries have been optimized for all systems.

  14. Density functional theory embedding for correlated wavefunctions: improved methods for open-shell systems and transition metal complexes.

    Science.gov (United States)

    Goodpaster, Jason D; Barnes, Taylor A; Manby, Frederick R; Miller, Thomas F

    2012-12-14

    Density functional theory (DFT) embedding provides a formally exact framework for interfacing correlated wave-function theory (WFT) methods with lower-level descriptions of electronic structure. Here, we report techniques to improve the accuracy and stability of WFT-in-DFT embedding calculations. In particular, we develop spin-dependent embedding potentials in both restricted and unrestricted orbital formulations to enable WFT-in-DFT embedding for open-shell systems, and develop an orbital-occupation-freezing technique to improve the convergence of optimized effective potential calculations that arise in the evaluation of the embedding potential. The new techniques are demonstrated in applications to the van-der-Waals-bound ethylene-propylene dimer and to the hexa-aquairon(II) transition-metal cation. Calculation of the dissociation curve for the ethylene-propylene dimer reveals that WFT-in-DFT embedding reproduces full CCSD(T) energies to within 0.1 kcal/mol at all distances, eliminating errors in the dispersion interactions due to conventional exchange-correlation (XC) functionals while simultaneously avoiding errors due to subsystem partitioning across covalent bonds. Application of WFT-in-DFT embedding to the calculation of the low-spin/high-spin splitting energy in the hexaaquairon(II) cation reveals that the majority of the dependence on the DFT XC functional can be eliminated by treating only the single transition-metal atom at the WFT level; furthermore, these calculations demonstrate the substantial effects of open-shell contributions to the embedding potential, and they suggest that restricted open-shell WFT-in-DFT embedding provides better accuracy than unrestricted open-shell WFT-in-DFT embedding due to the removal of spin contamination.

  15. Large-scale shell-model calculations of elastic and inelastic scattering rates of lightest supersymmetric particles (LSP) on I127, Xe129, Xe131, and Cs133 nuclei

    Science.gov (United States)

    Toivanen, P.; Kortelainen, M.; Suhonen, J.; Toivanen, J.

    2009-04-01

    We discuss the dark-matter detection rates for the elastic and inelastic scattering of the lightest supersymmetric particle (LSP) off nuclei. For this we use an easily accessible formalism where the underlying nuclear physics is condensed in structure coefficients multiplying the key parameters of supersymmetric theories. In this work we compute these coefficients for the stable iodine, xenon, and cesium nuclei by application of the nuclear shell model in a model space involving the 2s, 1d, 0g7/2, and 0h11/2 single-particle orbitals. As an interaction we use the renormalized Bonn-CD G matrix. By using fitted nuclear gyromagnetic factors we have successfully reproduced the relevant spectroscopic data on magnetic moments and M1 decays in the discussed nuclei.

  16. Application of critical COD and plastic instability concepts to fracture of shells. [Crack Opening Displacement

    Science.gov (United States)

    Erdogan, F.; Ratwani, M.

    1974-01-01

    The paper deals with the initiation, growth, and possible arrest of fracture in shell structures containing initial defects which may be approximated by an isolated part-through crack. The main study is restricted to the structures in which the net section of the shell wall around the defect zone is fully yielded. The problem is solved by using an 8th order shallow shell theory with a conventional plastic strip model to account for the plastic deformations. Using the critical COD or the plastic instability as fracture criterion, the results are applied to the fracture propagation and arrest in shells. The calculated results are then compared with those obtained from the experiments on zircaloy, aluminum, and steel pipes.

  17. Vibrations of an Elastic Orthotropic Unmoment Open Cylindrical Shell with Variable Curvature and Free End, when Other Edges are Rigid–Clamped

    Directory of Open Access Journals (Sweden)

    Ghulghazaryan G.R.

    2011-03-01

    Full Text Available The problem of existence of free vibrations of an elastic orthotropic open cylindrical shell (with arbitrary directional curve with free end, when other edges are rigid – clamped is studied. The investigation is carried out for elastic orthotropic shell when bending rigidity is vanishingly small (the moment free shell. The dispersion equations for finding the natural frequencies of vibrations are derived. The calculations were carried out for the shells with directing curve in form of a parabola with different values of curvature and lengths.

  18. Moderately large vibrations of doubly curved shallow open shells composed of thick layers

    Science.gov (United States)

    Adam, Christoph

    2007-02-01

    This paper addresses nonlinear flexural vibrations of shallow shells composed of three thick layers with different shear flexibility, which are symmetrically arranged with respect to the middle surface. The considered shell structures of polygonal planform are hard hinged simply supported (i.e. all in-plane rotations and the bending moment vanish) with the edges fully restraint against displacements in any direction. The kinematic field equations are formulated by layerwise application of a first-order shear deformation theory. A modification of Berger's theory is employed to model the nonlinear characteristics of the structural response. The continuity of the transverse shear stress across the interfaces is specified according to Hooke's law, and subsequently the equations of motion of this higher order problem can be derived in analogy to a homogeneous single-layer shear deformable shallow shell. Numerical results of rectangular shallow shells in nonlinear steady-state vibration are presented for various ratios of shell rise to thickness, and non-dimensional load amplitude.

  19. Assessment of the accuracy of coupled cluster perturbation theory for open-shell systems. II. Quadruples expansions

    Science.gov (United States)

    Eriksen, Janus J.; Matthews, Devin A.; Jørgensen, Poul; Gauss, Jürgen

    2016-05-01

    We extend our assessment of the potential of perturbative coupled cluster (CC) expansions for a test set of open-shell atoms and organic radicals to the description of quadruple excitations. Namely, the second- through sixth-order models of the recently proposed CCSDT(Q-n) quadruples series [J. J. Eriksen et al., J. Chem. Phys. 140, 064108 (2014)] are compared to the prominent CCSDT(Q) and ΛCCSDT(Q) models. From a comparison of the models in terms of their recovery of total CC singles, doubles, triples, and quadruples (CCSDTQ) energies, we find that the performance of the CCSDT(Q-n) models is independent of the reference used (unrestricted or restricted (open-shell) Hartree-Fock), in contrast to the CCSDT(Q) and ΛCCSDT(Q) models, for which the accuracy is strongly dependent on the spin of the molecular ground state. By further comparing the ability of the models to recover relative CCSDTQ total atomization energies, the discrepancy between them is found to be even more pronounced, stressing how a balanced description of both closed- and open-shell species—as found in the CCSDT(Q-n) models—is indeed of paramount importance if any perturbative CC model is to be of chemical relevance for high-accuracy applications. In particular, the third-order CCSDT(Q-3) model is found to offer an encouraging alternative to the existing choices of quadruples models used in modern computational thermochemistry, since the model is still only of moderate cost, albeit markedly more costly than, e.g., the CCSDT(Q) and ΛCCSDT(Q) models.

  20. Assessment of the accuracy of coupled cluster perturbation theory for open-shell systems. II. Quadruples expansions.

    Science.gov (United States)

    Eriksen, Janus J; Matthews, Devin A; Jørgensen, Poul; Gauss, Jürgen

    2016-05-21

    We extend our assessment of the potential of perturbative coupled cluster (CC) expansions for a test set of open-shell atoms and organic radicals to the description of quadruple excitations. Namely, the second- through sixth-order models of the recently proposed CCSDT(Q-n) quadruples series [J. J. Eriksen et al., J. Chem. Phys. 140, 064108 (2014)] are compared to the prominent CCSDT(Q) and ΛCCSDT(Q) models. From a comparison of the models in terms of their recovery of total CC singles, doubles, triples, and quadruples (CCSDTQ) energies, we find that the performance of the CCSDT(Q-n) models is independent of the reference used (unrestricted or restricted (open-shell) Hartree-Fock), in contrast to the CCSDT(Q) and ΛCCSDT(Q) models, for which the accuracy is strongly dependent on the spin of the molecular ground state. By further comparing the ability of the models to recover relative CCSDTQ total atomization energies, the discrepancy between them is found to be even more pronounced, stressing how a balanced description of both closed- and open-shell species-as found in the CCSDT(Q-n) models-is indeed of paramount importance if any perturbative CC model is to be of chemical relevance for high-accuracy applications. In particular, the third-order CCSDT(Q-3) model is found to offer an encouraging alternative to the existing choices of quadruples models used in modern computational thermochemistry, since the model is still only of moderate cost, albeit markedly more costly than, e.g., the CCSDT(Q) and ΛCCSDT(Q) models.

  1. Structure of neutron-rich nuclei around the N = 126 closed shell; the yrast structure of {sup 205}Au{sub 126} up to spin-parity I{sup {pi}} = (19/2{sup +})

    Energy Technology Data Exchange (ETDEWEB)

    Podolyak, Zs.; Steer, S.J.; Pietri, S.; Regan, P.H.; Brandau, C.; Catford, W.N.; Cullen, I.J.; Gelletly, W.; Jones, G.A.; Liu, Z.; Walker, P.M. [University of Surrey, Department of Physics, Guildford (United Kingdom); Gorska, M.; Gerl, J.; Wollersheim, H.J.; Grawe, H.; Becker, F.; Geissel, H.; Kelic, A.; Kojouharov, I.; Kurz, N.; Montes, F.; Prokopowicz, W.; Saito, T.; Schaffner, H.; Tashenov, S.; Werner-Malento, E. [GSI, Darmstadt (Germany); Rudolph, D.; Hoischen, R. [Lund University, Department of Physics, Lund (Sweden); Garnsworthy, A.B. [University of Surrey, Department of Physics, Guildford (United Kingdom); Yale University, WNSL, New Haven, CT (United States); Maier, K.H. [Institute of Nuclear Physics, Krakow (Poland); University of the West of Scotland, Dept. of Physics, Paisley (United Kingdom); Bednarczyk, P.; Grebosz, J. [GSI, Darmstadt (Germany); Institute of Nuclear Physics, Krakow (Poland); Caceres, L. [GSI, Darmstadt (Germany); Universidad Autonoma de Madrid, Dept. de Fisica Teorica, Madrid (Spain); Doornenbal, P. [GSI, Darmstadt (Germany); Universitaet zu Koeln, IKP, Koeln (Germany); Heinz, A. [Yale University, WNSL, New Haven, CT (United States); Kurtukian-Nieto, T. [Universidad de Santiago de Compostela, Santiago de Campostela (Spain); Benzoni, G.; Wieland, O. [Universita degli Studi di Milano (Italy); INFN, Milano (Italy); Pfuetzner, M. [Warsaw University, IEP, Warsaw (Poland); Jungclaus, A. [Universidad Autonoma de Madrid, Dept. de Fisica Teorica, Madrid (Spain); Balabanski, D.L. [Bulgarian Academy of Sciences, INRNE, Sofia (Bulgaria); Brown, B.A. [Univ. of Surrey, Dept. of Physics, Guildford (United Kingdom); Michigan State Univ., NSCL, East Lansing, MI (United States); Bruce, A.M.; Lalkovski, S. [Univ. of Brighton, School of Environment and Technology, Brighton (United Kingdom); Dombradi, Zs. [Institute for Nuclear Research, Debrecen (Hungary); Estevez, M.E. [Instituto de Fisica Corpuscular, Valencia (Spain)] [and others

    2009-12-15

    Heavy neutron-rich nuclei have been populated through the relativistic fragmentation of a {sup 208}{sub 82} Pb beam at E/A = 1 GeV on a 2.5 g/cm{sup 2} thick Be target. The synthesised nuclei were selected and identified in-flight using the fragment separator at GSI. Approximately 300 ns after production, the selected nuclei were implanted in an {proportional_to}8 mm thick perspex stopper, positioned at the centre of the RISING {gamma} -ray detector spectrometer array. A previously unreported isomer with a half-life T{sub 1/2} = 163(5) ns has been observed in the N=126 closed-shell nucleus {sup 205}{sub 79} Au. Through {gamma}-ray singles and {gamma}-{gamma} coincidence analysis a level scheme was established. The comparison with a shell model calculation tentatively identifies the spin-parity of the excited states, including the isomer itself, which is found to be I{sup {pi}} = (19/2{sup +}). (orig.)

  2. Direct observation of ring-opening dynamics in strong-field ionized selenophene using femtosecond inner-shell absorption spectroscopy

    Science.gov (United States)

    Lackner, Florian; Chatterley, Adam S.; Pemmaraju, C. D.; Closser, Kristina D.; Prendergast, David; Neumark, Daniel M.; Leone, Stephen R.; Gessner, Oliver

    2016-12-01

    Femtosecond extreme ultraviolet transient absorption spectroscopy is used to explore strong-field ionization induced dynamics in selenophene (C4H4Se). The dynamics are monitored in real-time from the viewpoint of the Se atom by recording the temporal evolution of element-specific spectral features near the Se 3d inner-shell absorption edge (˜58 eV). The interpretation of the experimental results is supported by first-principles time-dependent density functional theory calculations. The experiments simultaneously capture the instantaneous population of stable molecular ions, the emergence and decay of excited cation states, and the appearance of atomic fragments. The experiments reveal, in particular, insight into the strong-field induced ring-opening dynamics in the selenophene cation, which are traced by the emergence of non-cyclic molecules as well as the liberation of Se+ ions within an overall time scale of approximately 170 fs. We propose that both products may be associated with dynamics on the same electronic surfaces but with different degrees of vibrational excitation. The time-dependent inner-shell absorption features provide direct evidence for a complex relaxation mechanism that may be approximated by a two-step model, whereby the initially prepared, excited cyclic cation decays within τ1 = 80 ± 30 fs into a transient molecular species, which then gives rise to the emergence of bare Se+ and ring-open cations within an additional τ2 = 80 ± 30 fs. The combined experimental and theoretical results suggest a close relationship between σ* excited cation states and the observed ring-opening reactions. The findings demonstrate that the combination of femtosecond time-resolved core-level spectroscopy with ab initio estimates of spectroscopic signatures provide new insights into complex, ultrafast photochemical reactions such as ring-opening dynamics in organic molecules in real-time and with simultaneous sensitivity for electronic and structural

  3. Nuclear-electronic orbital reduced explicitly correlated Hartree-Fock approach: Restricted basis sets and open-shell systems

    Science.gov (United States)

    Brorsen, Kurt R.; Sirjoosingh, Andrew; Pak, Michael V.; Hammes-Schiffer, Sharon

    2015-06-01

    The nuclear electronic orbital (NEO) reduced explicitly correlated Hartree-Fock (RXCHF) approach couples select electronic orbitals to the nuclear orbital via Gaussian-type geminal functions. This approach is extended to enable the use of a restricted basis set for the explicitly correlated electronic orbitals and an open-shell treatment for the other electronic orbitals. The working equations are derived and the implementation is discussed for both extensions. The RXCHF method with a restricted basis set is applied to HCN and FHF- and is shown to agree quantitatively with results from RXCHF calculations with a full basis set. The number of many-particle integrals that must be calculated for these two molecules is reduced by over an order of magnitude with essentially no loss in accuracy, and the reduction factor will increase substantially for larger systems. Typically, the computational cost of RXCHF calculations with restricted basis sets will scale in terms of the number of basis functions centered on the quantum nucleus and the covalently bonded neighbor(s). In addition, the RXCHF method with an odd number of electrons that are not explicitly correlated to the nuclear orbital is implemented using a restricted open-shell formalism for these electrons. This method is applied to HCN+, and the nuclear densities are in qualitative agreement with grid-based calculations. Future work will focus on the significance of nonadiabatic effects in molecular systems and the further enhancement of the NEO-RXCHF approach to accurately describe such effects.

  4. Two-dimensional Penning ionization electron spectroscopy of open-shell metallocenes: outer valence ionic states of vanadocene and nickelocene.

    Science.gov (United States)

    Kishimoto, Naoki; Kimura, Miku; Ohno, Koichi

    2013-04-11

    In order to investigate outer valence ionic states of open-shell metallocenes, we have applied two-dimensional collision-energy/electron-energy-resolved Penning ionization electron spectroscopy (2D-PIES) upon collision with metastable He*(2(3)S) excited atoms as well as a high level ab initio molecular orbital calculation (the partial third-order quasiparticle theory of the electron propagator (P3)) to ionization from neutral ground states of vanadocene ((4)A2g) and nickelocene ((3)A2g). Assignments of observed Penning ionization electron/He I ultraviolet photoelectron spectra were consistent with the P3 calculation results for ionization of α and β spin electrons except for electron correlation bands observed by PIES. Negative collision energy dependence of partial Penning ionization cross-sections (CEDPICS) indicate attractive interaction with He*(2(3)S) around the molecule. Results by model potential calculation utilizing Li(2(2)S) instead of He*(2(3)S) for interaction between He*(2(3)S) and open-shell metallocenes do not explain the strong negative CEDPICS of the bands observed in PIES.

  5. Electronic fine structure calculation of metal complexes with three-open-shell s, d, and p configurations.

    Science.gov (United States)

    Ramanantoanina, Harry; Daul, Claude

    2017-08-01

    The ligand field density functional theory (LFDFT) algorithm is extended to treat the electronic structure and properties of systems with three-open-shell electron configurations, exemplified in this work by the calculation of the core and semi-core 1s, 2s, and 3s one-electron excitations in compounds containing transition metal ions. The work presents a model to non-empirically resolve the multiplet energy levels arising from the three-open-shell systems of non-equivalent ns, 3d, and 4p electrons and to calculate the oscillator strengths corresponding to the electric-dipole 3d (m)  → ns (1)3d (m) 4p (1) transitions, with n = 1, 2, 3 and m = 0, 1, 2, …, 10 involved in the s electron excitation process. Using the concept of ligand field, the Slater-Condon integrals, the spin-orbit coupling constants, and the parameters of the ligand field potential are determined from density functional theory (DFT). Therefore, a theoretical procedure using LFDFT is established illustrating the spectroscopic details at the atomic scale that can be valuable in the analysis and characterization of the electronic spectra obtained from X-ray absorption fine structure or electron energy loss spectroscopies.

  6. Evidence for Ultra-fast Outflows in Radio-quiet Active Galactic Nuclei. II. Detailed Photoionization Modeling of Fe K-shell Absorption Lines

    Science.gov (United States)

    Tombesi, F.; Cappi, M.; Reeves, J. N.; Palumbo, G. G. C.; Braito, V.; Dadina, M.

    2011-11-01

    X-ray absorption line spectroscopy has recently shown evidence for previously unknown Ultra-fast Outflows (UFOs) in radio-quiet active galactic nuclei (AGNs). These have been detected essentially through blueshifted Fe XXV/XXVI K-shell transitions. In the previous paper of this series we defined UFOs as those highly ionized absorbers with an outflow velocity higher than 10,000 km s-1 and assessed the statistical significance of the associated blueshifted absorption lines in a large sample of 42 local radio-quiet AGNs observed with XMM-Newton. The present paper is an extension of that work. First, we report a detailed curve of growth analysis of the main Fe XXV/XXVI transitions in photoionized plasmas. Then, we estimate an average spectral energy distribution for the sample sources and directly model the Fe K absorbers in the XMM-Newton spectra with the detailed Xstar photoionization code. We confirm that the frequency of sources in the radio-quiet sample showing UFOs is >35% and that the majority of the Fe K absorbers are indeed associated with UFOs. The outflow velocity distribution spans from ~10,000 km s-1 (~0.03c) up to ~100,000 km s-1 (~0.3c), with a peak and mean value of ~42,000 km s-1 (~0.14c). The ionization parameter is very high and in the range log ξ ~ 3-6 erg s-1 cm, with a mean value of log ξ ~ 4.2 erg s-1 cm. The associated column densities are also large, in the range N H ~ 1022-1024 cm-2, with a mean value of N H ~ 1023 cm-2. We discuss and estimate how selection effects, such as those related to the limited instrumental sensitivity at energies above 7 keV, may hamper the detection of even higher velocities and higher ionization absorbers. We argue that, overall, these results point to the presence of extremely ionized and possibly almost Compton-thick outflowing material in the innermost regions of AGNs. This also suggests that UFOs may potentially play a significant role in the expected cosmological feedback from AGNs and their study can

  7. Improvements to the on-line mass separator, RAMA, and the beta-delayed charged-particle emission of proton-rich sd shell nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Ognibene, Theodore Joseph [Lawrence Berkeley National Lab., CA (United States). Nuclear Science Div.

    1996-03-01

    To overcome the extreme difficulties encountered in the experimental decay studies of proton drip line nuclei, several techniques have been utilized, including a helium-jet transport system, particle identification detectors and mass separation. Improvements to the ion source/extraction region of the He-jet coupled on-line Recoil Atom Mass Analyzer (RAMA) and its target/ion source coupling resulted in significant increases in RAMA efficiencies and its mass resolution, as well as reductions in the overall transit time. At the 88-Inch Cyclotron at LBNL, the decays of 31Cl, 27P and 28P, with half-lives of 150 msec, 260 msec and 270.3 msec, respectively, were examined using a he-jet and low-energy gas ΔE-gas ΔE-silicon E detector telescopes. Total beta-delayed proton branches of 0.3% and 0.07% in 31Cl and 27P, respectively, were estimated. Several proton peaks that had been previously assigned to the decay of 31Cl were shown to be from the decay of 25Si. In 27P, two proton groups at 459 ± 14 keV and 610 ± 11 keV, with intensities of 7 ± 3% and 92 ± 4% relative to the main (100%) group were discovered. The Gamow-Teller component of the preceding beta-decay of each observed proton transition was compared to results from shell model calculations. Finally, a new proton transition was identified, following the β-decay of 28P, at 1,444 ± 12 keV with a 1.7 ± 0.5% relative intensity to the 100% group. Using similar low-energy detector telescopes and the mass separator TISOL at TRIUMF, the 109 msec and 173 msec activities, 17Ne and 33Ar, were studied. A new proton group with energy 729 ± 15 keV was observed following the beta-decay of 17Ne. Several discrepancies between earlier works as to the energies, intensities and assignments of several proton transitions from 17Ne and 33Ar were resolved.

  8. Improvements to the on-line mass separator, RAMA, and the beta-delayed charged-particle emission of proton-rich sd shell nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Ognibene, T.J. [Lawrence Berkeley National Lab., CA (United States). Nuclear Science Div.

    1996-03-01

    To overcome the extreme difficulties encountered in the experimental decay studies of proton drip line nuclei, several techniques have been utilized, including a helium-jet transport system, particle identification detectors and mass separation. Improvements to the ion source/extraction region of the He-jet coupled on-line Recoil Atom Mass Analyzer (RAMA) and its target/ion source coupling resulted in significant increases in RAMA efficiencies and its mass resolution, as well as reductions in the overall transit time. At the 88-Inch Cyclotron at LBNL, the decays of {sup 31}Cl, {sup 27}P and {sup 28}P, with half-lives of 150 msec, 260 msec and 270.3 msec, respectively, were examined using a he-jet and low-energy gas {Delta}E-gas {Delta}E-silicon E detector telescopes. Total beta-delayed proton branches of 0.3% and 0.07% in {sup 31}Cl and {sub 27}P, respectively, were estimated. Several proton peaks that had been previously assigned to the decay of {sup 31}Cl were shown to be from the decay of {sup 25}Si. In {sup 27}P, two proton groups at 459 {+-} 14 keV and 610 {+-} 11 keV, with intensities of 7 {+-} 3% and 92 {+-} 4% relative to the main (100%) group were discovered. The Gamow-Teller component of the preceding beta-decay of each observed proton transition was compared to results from shell model calculations. Finally, a new proton transition was identified, following the {beta}-decay of {sup 28}P, at 1,444 {+-} 12 keV with a 1.7 {+-} 0.5% relative intensity to the 100% group. Using similar low-energy detector telescopes and the mass separator TISOL at TRIUMF, the 109 msec and 173 msec activities, {sup 17}Ne and {sup 33}Ar, were studied. A new proton group with energy 729 {+-} 15 keV was observed following the beta-decay of {sup 17}Ne. Several discrepancies between earlier works as to the energies, intensities and assignments of several proton transitions from {sup 17}Ne and {sup 33}Ar were resolved.

  9. Hyper Open-Shell States: The Lowest Excited Spin States of O Atom, Fe(2+) Ion, and FeF2.

    Science.gov (United States)

    Varga, Zoltan; Verma, Pragya; Truhlar, Donald G

    2017-09-13

    Excited spin states are important for reactivity, catalysis, and magnetic applications. This work examines the relative energies of the spin states of O atom, Fe(2+) ion, and FeF2 and characterizes their excited spin states. Both single-configuration and multireference methods are used to establish the character of the lowest singlet excited state of all three systems and the lowest triplet excited state of Fe(2+) and FeF2. We find that the conventional representation of the orbital occupancies is incorrect in that the states have more unpaired electrons than the minimum number required by their total electron spin quantum number. In particular, we find that, for a given spin state, an electronic configuration with more than 2S unpaired electrons is more stable than the configuration with 2S unpaired electrons (where S is the spin of the system). For instance, triplet FeF2 with four unpaired electrons is lower in energy than triplet FeF2 with two unpaired electrons. Such highly open-shell configurations are labeled as hyper open-shell electronic configurations in this work and are compared to ordinary open-shell or closed-shell electronic configurations. The hyper open-shell states considered in this work are especially interesting because, unlike typical biradicals and polyradicals, the unpaired electrons are all on the same center. This work shows that the conventional perspective on spin-state energetics that usually assumes ordinary open shells for single-centered radicals needs modification to take into account, whenever possible, hyper open-shell configurations as well.

  10. Scattering Of Light Nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Quaglioni, S; Navratil, P; Roth, R

    2009-12-15

    The exact treatment of nuclei starting from the constituent nucleons and the fundamental interactions among them has been a long-standing goal in nuclear physics. Above all nuclear scattering and reactions, which require the solution of the many-body quantum-mechanical problem in the continuum, represent an extraordinary theoretical as well as computational challenge for ab initio approaches.We present a new ab initio many-body approach which derives from the combination of the ab initio no-core shell model with the resonating-group method [4]. By complementing a microscopic cluster technique with the use of realistic interactions, and a microscopic and consistent description of the nucleon clusters, this approach is capable of describing simultaneously both bound and scattering states in light nuclei. We will discuss applications to neutron and proton scattering on sand light p-shell nuclei using realistic nucleon-nucleon potentials, and outline the progress toward the treatment of more complex reactions.

  11. A state space solution for the bending problem of thick laminated piezoelectric open cylindrical shells

    Institute of Scientific and Technical Information of China (English)

    SHENG Hong-yu; LI He-ping; XU Hai-yan

    2009-01-01

    Based on the theories of three-dimensional elasticity and piezoelectricity, and by assuming appropriate boundary functions, we established a state equation of piezoelectric cylindrical shells. By using the transfer matrix method, we presented an analytical solution that satisfies all the arbitrary boundary conditions at boundary edges, as well as on upper and bottom surfaces. Our solution takes into account all the independent elastic and piezoelectric constants for a piezoelectric orthotropy, and satisfies continuity conditions between plies of the laminates. The principle of the present method and corresponding results can be widely used in many engineering fields and be applied to assess the effectiveness of varions approximate and numerical models.

  12. Selfconsistent calculations for hyperdeformed nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Molique, H.; Dobaczewski, J.; Dudek, J.; Luo, W.D. [Universite Louis Pasteur, Strasbourg (France)

    1996-12-31

    Properties of the hyperdeformed nuclei in the A {approximately} 170 mass range are re-examined using the self-consistent Hartree-Fock method with the SOP parametrization. A comparison with the previous predictions that were based on a non-selfconsistent approach is made. The existence of the {open_quotes}hyper-deformed shell closures{close_quotes} at the proton and neutron numbers Z=70 and N=100 and their very weak dependence on the rotational frequency is suggested; the corresponding single-particle energy gaps are predicted to play a role similar to that of the Z=66 and N=86 gaps in the super-deformed nuclei of the A {approximately} 150 mass range. Selfconsistent calculations suggest also that the A {approximately} 170 hyperdeformed structures have neglegible mass asymmetry in their shapes. Very importantly for the experimental studies, both the fission barriers and the {open_quotes}inner{close_quotes} barriers (that separate the hyperdeformed structures from those with smaller deformations) are predicted to be relatively high, up to the factor of {approximately}2 higher than the corresponding ones in the {sup 152}Dy superdeformed nucleus used as a reference.

  13. Finite Amplitude Method for Charge-Changing Transitions in Axially-Deformed Nuclei

    CERN Document Server

    Mustonen, M T; Zenginerler, Z; Engel, J

    2014-01-01

    We describe and apply a version of the finite amplitude method for obtaining the charge-changing nuclear response in the quasiparticle random phase approximation. The method is suitable for calculating strength functions and beta-decay rates, both allowed and forbidden, in axially-deformed open-shell nuclei. We demonstrate the speed and versatility of the code through a preliminary examination of the effects of tensor terms in Skyrme functionals on beta decay in a set of spherical and deformed open-shell nuclei. Like the isoscalar pairing interaction, the tensor terms systematically increase allowed beta-decay rates. This finding generalizes previous work in semimagic nuclei and points to the need for a comprehensive study of time-odd terms in nuclear density functionals.

  14. EUV magnetic-dipole lines from highly-charged high-Z ions with an open 3d shell

    CERN Document Server

    Osin, D; Reader, J; Ralchenko, Yu

    2012-01-01

    The electron beam ion trap (EBIT) at the National Institute of Standards and Technology was used to produce highly-charged ions of hafnium, tantalum and gold with an open 3d shell. The extreme-ultraviolet (EUV) spectra from these ions were recorded with a flat-field grazing-incidence spectrometer in the wavelength range of 4.5 nm to 25 nm. A total of 133 new spectral lines, primarily due to magnetic-dipole transitions within the ground-state $3d^n$ configurations of the Co-like to K-like ions, were identified by comparing energy-dependent experimental spectra with a detailed collisional-radiative modeling of the EBIT plasma.

  15. Shell model and spectroscopic factors

    Energy Technology Data Exchange (ETDEWEB)

    Poves, P. [Madrid Univ. Autonoma and IFT, UAM/CSIC, E-28049 (Spain)

    2007-07-01

    In these lectures, I introduce the notion of spectroscopic factor in the shell model context. A brief review is given of the present status of the large scale applications of the Interacting Shell Model. The spectroscopic factors and the spectroscopic strength are discussed for nuclei in the vicinity of magic closures and for deformed nuclei. (author)

  16. New high spin states and isomers in the {sup 208}Pb and {sup 207}Pb nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Broda, R.; Wrzesinski, J.; Pawlat, T. [and others

    1996-12-31

    The two most prominent examples of the heavy doubly closed shell (DCS) nuclei, {sup 208}Pb and {sup 132}Sn, are not accessible by conventional heavy-ion fusion processes populating high-spin states. This experimental difficulty obscured for a long time the investigation of yrast high-spin states in both DCS and neighboring nuclei and consequently restricted the study of the shell model in its most attractive regions. Recent technical development of multidetector gamma arrays opened new ways to exploit more complex nuclear processes which populate the nuclei of interest with suitable yields for gamma spectroscopy and involve population of moderately high spin states. This new possibility extended the range of accessible spin values and is a promising way to reach new yrast states. Some of these states are expected to be of high configurational purity and can be a source of important shell model parameters which possibly can be used later to check the validity of the spherical shell model description at yet higher spin and higher excitation energy. The nuclei in the closest vicinity of {sup 132}Sn are produced in spontaneous fission and states with spin values up to I=14 can be reached in fission gamma spectroscopy studies with the presently achieved sensitivity of gamma arrays. New results on yrast states in the {sup 134}Te and {sup 135}I nuclei populated in fission of the {sup 248}Cm presented at this conference illustrate such application of the resolving power offered by modern gamma techniques.

  17. A new near-linear scaling, efficient and accurate, open-shell domain-based local pair natural orbital coupled cluster singles and doubles theory.

    Science.gov (United States)

    Saitow, Masaaki; Becker, Ute; Riplinger, Christoph; Valeev, Edward F; Neese, Frank

    2017-04-28

    The Coupled-Cluster expansion, truncated after single and double excitations (CCSD), provides accurate and reliable molecular electronic wave functions and energies for many molecular systems around their equilibrium geometries. However, the high computational cost, which is well-known to scale as O(N(6)) with system size N, has limited its practical application to small systems consisting of not more than approximately 20-30 atoms. To overcome these limitations, low-order scaling approximations to CCSD have been intensively investigated over the past few years. In our previous work, we have shown that by combining the pair natural orbital (PNO) approach and the concept of orbital domains it is possible to achieve fully linear scaling CC implementations (DLPNO-CCSD and DLPNO-CCSD(T)) that recover around 99.9% of the total correlation energy [C. Riplinger et al., J. Chem. Phys. 144, 024109 (2016)]. The production level implementations of the DLPNO-CCSD and DLPNO-CCSD(T) methods were shown to be applicable to realistic systems composed of a few hundred atoms in a routine, black-box fashion on relatively modest hardware. In 2011, a reduced-scaling CCSD approach for high-spin open-shell unrestricted Hartree-Fock reference wave functions was proposed (UHF-LPNO-CCSD) [A. Hansen et al., J. Chem. Phys. 135, 214102 (2011)]. After a few years of experience with this method, a few shortcomings of UHF-LPNO-CCSD were noticed that required a redesign of the method, which is the subject of this paper. To this end, we employ the high-spin open-shell variant of the N-electron valence perturbation theory formalism to define the initial guess wave function, and consequently also the open-shell PNOs. The new PNO ansatz properly converges to the closed-shell limit since all truncations and approximations have been made in strict analogy to the closed-shell case. Furthermore, given the fact that the formalism uses a single set of orbitals, only a single PNO integral transformation is

  18. Tentative study of nuclear charge radii for neutron-deficient nuclei around the Z = 82 shell from experimental α decay data

    Energy Technology Data Exchange (ETDEWEB)

    Qian, Yibin, E-mail: qyibin@njust.edu.cn [Department of Applied Physics, Nanjing University of Science and Technology, Nanjing 210094 (China); Department of Physics and Key Laboratory of Modern Acoustics, Nanjing University, Nanjing 210093 (China); Ren, Zhongzhou [Department of Physics and Key Laboratory of Modern Acoustics, Nanjing University, Nanjing 210093 (China); Center of Theoretical Nuclear Physics, National Laboratory of Heavy-Ion Accelerator, Lanzhou 730000 (China); Kavli Institute for Theoretical Physics China, Beijing 100190 (China)

    2016-01-15

    We tentatively investigate the root-mean-square (rms) nuclear charge radii of odd-A Po and Pb isotopes plus Tl isotopes, particularly concerning these difficultly-detected nuclei along with short lifetimes, via various data on α decay. Within the density-dependent cluster model, the density distributions of studied daughter nuclei are determined by exactly reproducing the corresponding experimental α decay half-lives, which leads the final results of nuclear charge radii. In addition, our recently proposed formula deducing the charge radii is extended to this study for comparison. Whether it concerns the ground or isomeric state of target nuclei, the extracted nuclear charge radii are found to be in good agreement with the measured values. Sequential predictions on the rms charge radii are subsequently made for these neutron-deficient nuclei and especially for the rarely detected Bi isotopic chain, which are expected to be useful for future measurements. Moreover, the variety of α-preformation factors is analyzed in the scheme of valence nucleon number to pursue the further improvement of the model. This may be considered as an effective effort to obtain the charge radii of ground and even low-lying excited states for exotic nuclei near the proton-dripline.

  19. Proxy-SU(3) symmetry in heavy deformed nuclei

    Science.gov (United States)

    Bonatsos, Dennis; Assimakis, I. E.; Minkov, N.; Martinou, Andriana; Cakirli, R. B.; Casten, R. F.; Blaum, K.

    2017-06-01

    Background: Microscopic calculations of heavy nuclei face considerable difficulties due to the sizes of the matrices that need to be solved. Various approximation schemes have been invoked, for example by truncating the spaces, imposing seniority limits, or appealing to various symmetry schemes such as pseudo-SU(3). This paper proposes a new symmetry scheme also based on SU(3). This proxy-SU(3) can be applied to well-deformed nuclei, is simple to use, and can yield analytic predictions. Purpose: To present the new scheme and its microscopic motivation, and to test it using a Nilsson model calculation with the original shell model orbits and with the new proxy set. Method: We invoke an approximate, analytic, treatment of the Nilsson model, that allows the above vetting and yet is also transparent in understanding the approximations involved in the new proxy-SU(3). Results: It is found that the new scheme yields a Nilsson diagram for well-deformed nuclei that is very close to the original Nilsson diagram. The specific levels of approximation in the new scheme are also shown, for each major shell. Conclusions: The new proxy-SU(3) scheme is a good approximation to the full set of orbits in a major shell. Being able to replace a complex shell model calculation with a symmetry-based description now opens up the possibility to predict many properties of nuclei analytically and often in a parameter-free way. The new scheme works best for heavier nuclei, precisely where full microscopic calculations are most challenged. Some cases in which the new scheme can be used, often analytically, to make specific predictions, are shown in a subsequent paper.

  20. MOLECULAR OPEN-SHELL CONFIGURATION-INTERACTION CALCULATIONS USING THE DIRAC-COULOMB HAMILTONIAN - THE F6-MANIFOLD OF AN EMBEDDED EUO69- CLUSTER

    NARCIS (Netherlands)

    VISSER, O; VISSCHER, L; AERTS, PJC; NIEUWPOORT, WC

    1992-01-01

    We present results of all-electron molecular relativistic (Hartree-Fock-Dirac) and nonrelativistic (Hartree-Fock) calculations followed by a complete open shell configuration interaction (COSCI) calculation on an EuO6(9-) cluster in a Ba2GdNbO6 crystal. The results include the calculated energies of

  1. MOLECULAR OPEN-SHELL CONFIGURATION-INTERACTION CALCULATIONS USING THE DIRAC-COULOMB HAMILTONIAN - THE F6-MANIFOLD OF AN EMBEDDED EUO69- CLUSTER

    NARCIS (Netherlands)

    VISSER, O; VISSCHER, L; AERTS, PJC; NIEUWPOORT, WC

    1992-01-01

    We present results of all-electron molecular relativistic (Hartree-Fock-Dirac) and nonrelativistic (Hartree-Fock) calculations followed by a complete open shell configuration interaction (COSCI) calculation on an EuO6(9-) cluster in a Ba2GdNbO6 crystal. The results include the calculated energies of

  2. Spectroscopic Studies of Exotic Nuclei at ISOLDE

    CERN Multimedia

    2002-01-01

    Experiment IS50 is designed to: a) Investigate the full range of the @b strength function of heavy (A~$>$~48)~K nuclei b)~Study the decay of isomeric states in n-deficient bromine nuclei (A~=~72 and 70). The heavy K isotopes appeared to have complex decay schemes, including feeding by the @b-decay of levels having open neutron channels (Beta decay energy Q(@b) exceeds neutron binding energy S^n); in addition, a large fraction of the delayed transitions populate excited levels in the daughter nuclei. The allowed @b-decay selects states in the daughter nucleus with wave functions having a large overlap with the initial state. Hence, the @b strength functions, deduced from these deca reveal simple structures correlated to the particle-hole excitation energies in the Ca nuclei. These results are valuable for the application of the shell-model calculations far from stability. The delayed neutron spectra are measured with a large area curved scintillator in coincidence either with high resolution Ge(Li) detectors, ...

  3. Off-shell scalar products for the XXZ spin chain with open boundaries

    Directory of Open Access Journals (Sweden)

    W. Galleas

    2015-04-01

    Full Text Available In this work we study scalar products of Bethe vectors associated with the XXZ spin chain with open boundary conditions. The scalar products are obtained as solutions of a system of functional equations. The description of scalar products through functional relations follows from a particular map having the reflection algebra as its domain and a function space as the codomain. Within this approach we find a multiple contour integral representation for the scalar products in which the homogeneous limit can be obtained trivially.

  4. Third-order nonlinear optical properties of open-shell supermolecular systems composed of acetylene linked phenalenyl radicals.

    Science.gov (United States)

    Nakano, Masayoshi; Kishi, Ryohei; Yoneda, Kyohei; Inoue, Yudai; Inui, Tomoya; Shigeta, Yasuteru; Kubo, Takashi; Champagne, Benoît

    2011-08-11

    toward designing a variety of open-shell NLO supermolecular systems composed of phenalenyl radical building blocks.

  5. Study of shell closures N=40 and N=50 in neutron-rich nuclei; Etude des fermetures de couches N=40 et N=50 dans les noyaux riches en neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Perru, O

    2004-12-01

    For this thesis I have studied 2 neutron shell closures: N=40 and N=50. On N=50, an experiment was done in February 2001 on the ISOL line PARRNe, the issue was to measure the first excited states of {sup 83}Ge (Z=32, N=51) by studying the beta decay of {sup 83}Ga produced by fission of {sup 238}U.The extreme precision of the experimental device, with the operation of hot plasma ion sources made it possible to reach spectroscopic information of the Ge isotopes beyond the magic gap N=50. Two transitions have been attributed to {sup 83}Ge: at 867 keV and at 1238 keV. The level scheme of {sup 83}Ge could be interpreted in terms of weak coupling: the excited states of this nucleus are due to the couplings between the single neutron beyond N=50 and the remaining nucleons.On N=40, we wanted to determine the transition probability between ground state and first excited state, called B(E2), in {sup 70}Ni (N=42) and {sup 74}Zn (N=44) from Coulomb excitation. These exotic nuclei are produced by fragmentation of a primary beam of {sup 76}Ge on a target of {sup 58}Ni, selected by the spectrometer LISE, then interact with a secondary {sup 208}Pb target to induce the Coulomb excitation. At the end of this analysis, the following values have been obtained: B(E2,{sup 70}Ni)=860(170) e{sup 2}fm{sup 4}, B(E2,{sup 74}Zn)=1960(140) e{sup 2}fm{sup 4}. These values have been compared on the one hand to variational calculations which I have realised, on the other hand to published shell model calculations.These calculations point out the complex aspect of the Ni nuclei, which do not seem to have a typical behaviour of semi magic nuclei although they are located on a closed shell in protons (Z=28). (author)

  6. Symmetries in Nuclei

    CERN Document Server

    Van Isacker, P

    2010-01-01

    The use of dynamical symmetries or spectrum generating algebras for the solution of the nuclear many-body problem is reviewed. General notions of symmetry and dynamical symmetry in quantum mechanics are introduced and illustrated with simple examples such as the SO(4) symmetry of the hydrogen atom and the isospin symmetry in nuclei. Two nuclear models, the shell model and the interacting boson model, are reviewed with particular emphasis on their use of group-theoretical techniques.

  7. Dynamic Properties of Viscoelastic Open Shallow Shells%粘弹性开敞浅壳的动力学性质

    Institute of Scientific and Technical Information of China (English)

    2000-01-01

    On the basis of the Kármán-Donnell theory of thin shells with large deflections and the Boltzmann laws for linear viscoelastic materials, the mathematical model for viscoelastic open shallow shells was formulated. By using the Galerkin average method, the original integro-partial-differential dynamic system was simplified as a integro-ordinary-differential dynamic system, which can be transformed into a ordinary differential dynamic system by introducing new variables. The dynamical behavior was studied by some classical methods. Dynamical properties, such as, chaos, strange attractor, limit cycle etc., were discovered.

  8. Low-energy Dipole Excitations in Nuclei at the N=50,82 and Z=50 Shell Closures as Signatures for a Neutron Skin

    CERN Document Server

    Tsoneva, N

    2007-01-01

    Low-energy dipole excitations have been investigated theoretically in N=50, several N=82 isotones and the Z=50 Sn isotopes. For this purpose a method incorporating both HFB and multi-phonon QPM theory is applied. A concentration of one-phonon dipole strength located below the neutron emission threshold has been calculated in these nuclei. The analysis of the corresponding neutron and proton dipole transition densities allows to assign a genuine pattern to the low-energy excitations and making them distinct from the conventional GDR modes. Analyzing also the QRPA wave functions of the states we can identify these excitations as Pygmy Dipole Resonance (PDR) modes, recently studied also in Sn and N=82 nuclei. The results for N=50 are exploratory for an experimental project designed for the bremsstrahlung facility at the ELBE accelerator.

  9. Relativistic equation-of-motion coupled-cluster method using open-shell reference wavefunction: Application to ionization potential

    Science.gov (United States)

    Pathak, Himadri; Sasmal, Sudip; Nayak, Malaya K.; Vaval, Nayana; Pal, Sourav

    2016-08-01

    The open-shell reference relativistic equation-of-motion coupled-cluster method within its four-component description is successfully implemented with the consideration of single- and double- excitation approximations using the Dirac-Coulomb Hamiltonian. At the first attempt, the implemented method is employed to calculate ionization potential value of heavy atomic (Ag, Cs, Au, Fr, and Lr) and molecular (HgH and PbF) systems, where the effect of relativity does really matter to obtain highly accurate results. Not only the relativistic effect but also the effect of electron correlation is crucial in these heavy atomic and molecular systems. To justify the fact, we have taken two further approximations in the four-component relativistic equation-of-motion framework to quantify how the effect of electron correlation plays a role in the calculated values at different levels of theory. All these calculated results are compared with the available experimental data as well as with other theoretically calculated values to judge the extent of accuracy obtained in our calculations.

  10. Assessment of the accuracy of coupled cluster perturbation theory for open-shell systems. II. Quadruples expansions

    CERN Document Server

    Eriksen, Janus J; Jørgensen, Poul; Gauss, Jürgen

    2016-01-01

    We extend our assessment of the potential of perturbative coupled cluster (CC) expansions for a test set of open-shell species to the description of quadruple excitations. In doing so, we compare the prominent CCSDT(Q) and lambda-CCSDT(Q) (a-CCSDT(Q)) models, in which the CC singles, doubles, and triples (CCSDT) energy is augmented by similar corrections for quadruple excitations, to the second- through sixth-order models of the CCSDT(Q-n) quadruples series, which is based on a CCSDT rather than an HF zeroth-order state. By comparing the models in terms of the size-intensive recovery of as well as the total deviation from the quadruples contribution to CC singles, doubles, triples, and quadruples (CCSDTQ) energies, we find (i) that the accuracy offered by the CCSDT(Q) and a-CCSDT(Q) models is strongly dependent on the spin of the molecular ground state - like for the CCSD(T) model in the first part of the present series [arXiv:1512.02846] - and (ii) that the performance of the CCSDT(Q-n) models is practically...

  11. Density functional theory embedding for correlated wavefunctions: Improved methods for open-shell systems and transition metal complexes

    CERN Document Server

    Goodpaster, Jason D; Manby, Frederick R; Miller, Thomas F

    2012-01-01

    Density functional theory (DFT) embedding provides a formally exact framework for interfacing correlated wave-function theory (WFT) methods with lower-level descriptions of electronic structure. Here, we report techniques to improve the accuracy and stability of WFT-in-DFT embedding calculations. In particular, we develop spin-dependent embedding potentials in both restricted and unrestricted orbital formulations to enable WFT-in-DFT embedding for open-shell systems, and we develop an orbital-occupation-freezing technique to improve the convergence of optimized effective potential (OEP) calculations that arise in the evaluation of the embedding potential. The new techniques are demonstrated in applications to the van-der-Waals-bound ethylene-propylene dimer and to the hexaaquairon(II) transition-metal cation. Calculation of the dissociation curve for the ethylene-propylene dimer reveals that WFT-in-DFT embedding reproduces full CCSD(T) energies to within 0.1 kcal/mol at all distances, eliminating errors in th...

  12. Natural orbitals representation and Fermi sea depletion in finite nuclei and nuclear matter

    CERN Document Server

    Psonis, V P; Massen, S E

    2013-01-01

    The natural orbitals and natural occupation numbers of various N = Z, sp and sd shell nuclei are calculated by applying a correlated one-body density matrix. The correlated density matrix has been evaluated by considering central correlations of Jastrow type and an approximation named factor cluster expansion. The correlation effects on the natural orbitals, natural occupation numbers and the Fermi sea depletion are discussed and analysed. In addition, an approximate expression for the correlated one-body density matrix of the nuclear matter has been used for the evaluation of the relative momentum distribution and the Fermi sea depletion. We found that the value of the Fermi sea depletion is higher in closed shell nuclei compared to open shell ones and it is lower compared to the case of nuclear matter. This statement could be confirmed by relevant experimental studies.

  13. The effect of gap in n(k, ρ) on the single-particle properties of nucleons and the ground-state binding energy of closed-shell nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Mariji, H. [University of Coimbra, Centro de Fisica Computacional, Department of Physics, Coimbra (Portugal)

    2016-04-15

    The present work evaluates the effect of gap in the density-dependent one-body momentum distribution, n(k, ρ), at the Fermi surface on the calculation of the single-particle properties of nucleons, i.e., the momentum- and density-dependent single-particle potential and the nucleon effective mass, and also on the calculation of the ground-state binding energy of the selected closed-shell nuclei, i.e., {sup 16}O, {sup 40}Ca, and {sup 56}Ni. In order to do this, n(k, ρ) is constructed by use of the calculations of the lowest-order constrained variational method for the symmetric nuclear matter with the Av{sub 18} potential up to J{sub max} = 2 and 5. It is shown that the gap in n(k, ρ) at the Fermi surface has no significant effect on the calculation of single-particle properties in the case of J{sub max} = 5. In the relevant evaluation of the ground-state binding energy of selected nuclei, it is seen that the binding energy of {sup 16}O, improved by including n(k, ρ), is closer to the experimental data, contrary to {sup 40}Ca and {sup 56}Ni. (orig.)

  14. Spontaneous fission of superheavy nuclei

    Indian Academy of Sciences (India)

    R A Gherghescu; D N Poenaru

    2015-09-01

    The macroscopic–microscopic method is extended to calculate the deformation energy and penetrability for binary nuclear configurations typical for fission processes. The deformed two-centre shell model is used to obtain single-particle energy levels for the transition region of two partially overlapped daughter and emitted fragment nuclei. The macroscopic part is obtained using the Yukawa-plus-exponential potential. The microscopic shell and pairing corrections are obtained using the Strutinsky and BCS approaches and the cranking formulae yield the inertia tensor. Finally, the WKB method is used to calculate penetrabilities and spontaneous fission half-lives. Calculations are performed for the decay of 282,292120 nuclei.

  15. Electron capture and beta-decay rates for sd-shell nuclei in stellar environments relevant to high density O-Ne-Mg cores

    CERN Document Server

    Suzuki, Toshio; Nomoto, Ken'ichi

    2015-01-01

    Electron capture and beta-decay rates for nuclear pairs in sd-shell are evaluated at high densities and high temperatures relevant to the final evolution of electron-degenerate O-Ne-Mg cores of stars with the initial masses of 8-10 solar mass. Electron capture induces a rapid contraction of the electron-degenerate O-Ne-Mg core. The outcome of rapid contraction depends on the evolutionary changes in the central density and temperature, which are determined by the competing processes of contraction, cooling, and heating. The fate of the stars are determined by these competitions, whether they end up with electron-capture supernovae or Fe core-collapse supernovae. Since the competing processes are induced by electron capture and beta-decay, the accurate weak rates are crucially important. The rates are obtained for pairs with A=20, 23, 24, 25 and 27 by shell-model calculations in sd-shell with the USDB Hamiltonian. Effects of Coulomb corrections on the rates are evaluated. The rates for pairs with A=23 and 25 ar...

  16. Multi-shell effective interactions

    CERN Document Server

    Tsunoda, Naofumi; Hjorth-Jensen, Morten; Otsuka, Takaharu

    2013-01-01

    Background: Effective interactions, either derived from microscopic theories or based on fitting selected properties of nuclei in specific mass regions, are widely used inputs to shell-model studies of nuclei. Until recently, most shell-model calculations have been confined to a single oscillator shell. Recent interest in nuclei away from the stability line, requires however larger shell-model spaces. Since the derivation of microscopic effective interactions has been limited to degenerate model spaces, there are both conceptual and practical limits to present shell-model calculations that utilize such interactions. Purpose: The aim of this work is to present a novel microscopic method to calculate effective interactions for the nuclear shell model. Its main difference from existing theories is that it can be applied not only to degenerate model spaces but also to non-degenerate model spaces. Methods: The formalism is presented in the form of many-body perturbation theory based on the recently developed Exten...

  17. Evaluation of Orbital-and Ground State Energies of Some Open-and Closed-Shell Atoms over Integer and Noninteger Slater Type Orbitals

    Institute of Scientific and Technical Information of China (English)

    YAKAR,Yusuf

    2007-01-01

    Ab initio calculations of the orbital and the ground state energies of some open- and closed-shell atoms over Slater type orbitals with quantum numbers integer and Slater type orbitals with quantum numbers noninteger have been performed. In order to increase the efficiency of these calculations the atomic two-electron integrals were expressed in terms of incomplete beta function. Results were observed to be in good agreement with the literature.

  18. ELECTRON-CAPTURE AND β-DECAY RATES FOR sd-SHELL NUCLEI IN STELLAR ENVIRONMENTS RELEVANT TO HIGH-DENSITY O–NE–MG CORES

    Energy Technology Data Exchange (ETDEWEB)

    Suzuki, Toshio [Department of Physics and Graduate School of Integrated Basic Sciences, College of Humanities and Sciences, Nihon University Sakurajosui 3-25-40, Setagaya-ku, Tokyo 156-8550 (Japan); Toki, Hiroshi [Research Center for Nuclear Physics (RCNP), Osaka University, Ibaraki, Osaka 567-0047 (Japan); Nomoto, Ken’ichi, E-mail: suzuki@phys.chs.nihon-u.ac.jp [Kavli Institute for the Physics and Mathematics of the Universe (WPI), The University of Tokyo, Kashiwa, Chiba 277-8583 (Japan)

    2016-02-01

    Electron-capture and β-decay rates for nuclear pairs in the sd-shell are evaluated at high densities and high temperatures relevant to the final evolution of electron-degenerate O–Ne–Mg cores of stars with initial masses of 8–10 M{sub ⊙}. Electron capture induces a rapid contraction of the electron-degenerate O–Ne–Mg core. The outcome of rapid contraction depends on the evolutionary changes in the central density and temperature, which are determined by the competing processes of contraction, cooling, and heating. The fate of the stars is determined by these competitions, whether they end up with electron-capture supernovae or Fe core-collapse supernovae. Since the competing processes are induced by electron capture and β-decay, the accurate weak rates are crucially important. The rates are obtained for pairs with A = 20, 23, 24, 25, and 27 by shell-model calculations in the sd-shell with the USDB Hamiltonian. Effects of Coulomb corrections on the rates are evaluated. The rates for pairs with A = 23 and 25 are important for nuclear Urca processes that determine the cooling rate of the O–Ne–Mg core, while those for pairs with A = 20 and 24 are important for the core contraction and heat generation rates in the core. We provide these nuclear rates at stellar environments in tables with fine enough meshes at various densities and temperatures for studies of astrophysical processes sensitive to the rates. In particular, the accurate rate tables are crucially important for the final fates of not only O–Ne–Mg cores but also a wider range of stars, such as C–O cores of lower-mass stars.

  19. Third-Order Incremental Dual-Basis Set Zero-Buffer Approach for Large High-Spin Open-Shell Systems.

    Science.gov (United States)

    Zhang, Jun; Dolg, Michael

    2015-03-10

    The third-order incremental dual-basis set zero-buffer approach (inc3-db-B0) is an efficient, accurate, and black-box quantum chemical method for obtaining correlation energies of large systems, and it has been successfully applied to many real chemical problems. In this work, we extend this approach to high-spin open-shell systems. In the open-shell approach, we will first decompose the occupied orbitals of a system into several domains by a K-means clustering algorithm. The essential part is that we preserve the active (singly occupied) orbitals in all the calculations of the domain correlation energies. The duplicated contributions of the active orbitals to the correlation energy are subtracted from the incremental expansion. All techniques of truncating the virtual space such as the B0 approximation can be applied. This open-shell inc3-db-B0 approach is combined with the CCSD and CCSD(T) methods and applied to the computations of a singlet-triplet gap and an electron detachment process. Our approach exhibits an accuracy better than 0.6 kcal/mol or 0.3 eV compared with the standard implementation, while it saves a large amount of the computational time and can be efficiently parallelized.

  20. Critical Assessment of Time-Dependent Density Functional Theory for Excited States of Open-Shell Systems: II. Doublet-Quartet Transitions.

    Science.gov (United States)

    Li, Zhendong; Liu, Wenjian

    2016-06-14

    Compared with closed-shell systems, open-shell systems place three additional challenges to time-dependent density functional theory (TD-DFT) for electronically excited states: (a) the spin-contamination problem is a serious issue; (b) the exchange-correlation (XC) kernel may be numerically instable; and (c) the single-determinant description of open-shell ground states readily becomes energetically instable. Confined to flip-up single excitations, the spin-contamination problem can largely be avoided by using the spin-flip TD-DFT (SF-TD-DFT) formalism, provided that a noncollinear XC kernel is employed. As for the numerical instabilities associated with such a kernel, only an ad hoc scheme has been proposed so far, viz., the ALDA0 kernel, which amounts to setting the divergent components (arising from density gradients and kinetic energy density) simply to zero. The ground-state instability problem can effectively be avoided by introducing the Tamm-Dancoff approximation (TDA) to TD-DFT. Therefore, on a general basis, the SF-TDA/ALDA0 Ansatz is so far the only promising means within the TD-DFT framework for flip-up single excitations of open-shell systems. To assess systematically the performance of SF-TDA/ALDA0, in total 61 low-lying quartet excited states of the benchmark set of 11 small radicals [J. Chem. Theory Comput. 2016, 12, 238] are investigated with various XC functionals. Taking the MRCISD+Q (multireference configuration interaction with singles and doubles plus the Davidson correction) results as benchmark, it is found that the mean absolute errors of SF-TDA/ALDA0 with the SAOP (statistical averaging of model orbital potentials), global hybrid, and range-separated hybrid functionals are in the range of 0.2-0.4 eV. This is in line not only with the typical accuracy of TD-DFT for singlet and triplet excited states of closed-shell systems but also with the gross accuracy of spin-adapted TD-DFT for spin-conserving excited states of open-shell systems.

  1. Fusion excitation functions involving transitional nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Rehm, K.E.; Jiang, C.L.; Esbensen, H. [and others

    1995-08-01

    Measurements of fusion excitation functions involving transitional nuclei {sup 78}Kr and {sup 100}Mo showed a different behavior at low energies, if compared to measurements with {sup 86}Kr and {sup 92}Mo. This points to a possible influence of nuclear structure on the fusion process. One way to characterize the structure of vibrational nuclei is via their restoring force parameters C{sub 2} which can be calculated from the energy of the lowest 2{sup +} state and the corresponding B(E2) value. A survey of the even-even nuclei between A = 28-150 shows strong variations in C{sub 2} values spanning two orders of magnitude. The lowest values for C{sub 2} are observed for {sup 78}Kr, {sup 104}Ru and {sup 124}Xe followed by {sup 74,76}Ge, {sup 74,76}Se, {sup 100}Mo and {sup 110}Pd. In order to learn more about the influence of {open_quotes}softness{close_quotes} on the sub-barrier fusion enhancement, we measured cross sections for evaporation residue production for the systems {sup 78}Kr + {sup 104}Ru and {sup 78}Kr + {sup 76}Ge with the gas-filled magnet technique. For both systems, fusion excitation functions involving the closed neutron shell nucleus {sup 86}Kr were measured previously. The data are presently being analyzed.

  2. Investigation of doublet-bands in {sup 124,126,130,132}Cs odd–odd nuclei using triaxial projected shell model approach

    Energy Technology Data Exchange (ETDEWEB)

    Bhat, G.H.; Ali, R.N. [Department of Physics, University of Kashmir, Srinagar, 190 006 (India); Sheikh, J.A. [Department of Physics, University of Kashmir, Srinagar, 190 006 (India); Department of Physics and Astronomy, University of Tennessee, Knoxville, TN 37996 (United States); Palit, R. [Department of Nuclear and Atomic Physics, Tata Institute of Fundamental Research, Colaba, Mumbai, 400 005 (India)

    2014-02-15

    Doublet bands observed in {sup 124,126,130,132}Cs isotopes are studied using the recently developed multi-quasiparticle microscopic triaxial projected shell model (TPSM) approach. It is shown that TPSM results for energies and transition probabilities are in good agreement with known energies and the recently measured extensive data on transition probabilities for the bands in {sup 126}Cs. In particular, it is demonstrated that characteristics transition probabilities expected for the doublet bands to originate from the chiral symmetry breaking are well reproduced in the present work. The calculated energies for {sup 124,130,132}Cs are also shown to be in reasonable agreement with the available experimental data. Furthermore, a complete set of the calculated transition probabilities is provided for the doublet bands in {sup 124,130,132}Cs isotopes.

  3. Density-fitted open-shell symmetry-adapted perturbation theory and application to π-stacking in benzene dimer cation and ionized DNA base pair steps

    Science.gov (United States)

    Gonthier, Jérôme F.; Sherrill, C. David

    2016-10-01

    Symmetry-Adapted Perturbation Theory (SAPT) is one of the most popular approaches to energy component analysis of non-covalent interactions between closed-shell systems, yielding both accurate interaction energies and meaningful interaction energy components. In recent years, the full open-shell equations for SAPT up to second-order in the intermolecular interaction and zeroth-order in the intramolecular correlation (SAPT0) were published [P. S. Zuchowski et al., J. Chem. Phys. 129, 084101 (2008); M. Hapka et al., ibid. 137, 164104 (2012)]. Here, we utilize density-fitted electron repulsion integrals to produce an efficient computational implementation. This approach is used to examine the effect of ionization on π-π interactions. For the benzene dimer radical cation, comparison against reference values indicates a good performance for open-shell SAPT0, except in cases with substantial charge transfer. For π stacking between hydrogen-bonded pairs of nucleobases, dispersion interactions still dominate binding, in spite of the creation of a positive charge.

  4. Ab Initio Exploration of the Potential Energy Surface of the O_2-SO_2 Open-Shell Complex.

    Science.gov (United States)

    Fawzy, Wafaa M.; Hougen, Jon T.

    2016-06-01

    The O_2-SO_2 complex is believed to be a precursor to acid rain. The previously observed FTMW spectrum suggested internal motions within the complex, but their nature was not identified. Development of an effective Hamiltonian for an open-shell molecule with tunneling requires knowledge of the potential energy surface (PES) and the intrinsic reaction coordinates (IRC) for the paths between minima. A recent ab initio study reported two different nonplanar minima in the ground electronic state of O_2-SO_2. These predictions were based on geometry optimization calculations at the MP2/aug-cc-pVnZ level of theory, with n = 2 and 3. The current work is focused on a highly correlated ab initio investigation of the global PES (a 9-D problem) in the ground triplet electronic state of O_2-SO_2. Because of the high dimensionality in the complex, the PES calculations are partitioned into several two-dimensional cuts through the PES. We have so far explored only a 3-D part of the global PES to look for stable planar configurations. These calculations included geometry optimization, frequency, and single point energy calculations. Calculations were performed using UCCSD(T)/aug-cc-pV(n+D)Z,where n = 2 and 3, level of theory. We used an axis system that defines the radial and the angular van der Waals coordinates for a planar complex as RvW, θ_1, and θ_2. The bond length (RvW) is the distance between the center of mass of the O_2 unit and the S atom. θ_1 and θ_2 are the angles between the van der Waals bond and the O_2 internuclear axis or one of the SO bonds in the SO_2 moiety, respectively. Full geometry optimization calculations predicted a minimum of C_s symmetry in which both the O_2 and SO_2 units are tilted with respect to the van der Waals bond, and RvW = 3.63 {Å}. 3-D PES surface calculations, which involve the RvW, θ_1, and θ_2 vdW coordinates, showed that the optimized structure is the global minimum. In addition, a local minimum at RvW = 3.9 {Å}, which

  5. Density Functional Theory of Open-Shell Systems. The 3d-Series Transition-Metal Atoms and Their Cations.

    Science.gov (United States)

    Luo, Sijie; Averkiev, Boris; Yang, Ke R; Xu, Xuefei; Truhlar, Donald G

    2014-01-14

    The 3d-series transition metals (also called the fourth-period transition metals), Sc to Zn, are very important in industry and biology, but they provide unique challenges to computing the electronic structure of their compounds. In order to successfully describe the compounds by theory, one must be able to describe their components, in particular the constituent atoms and cations. In order to understand the ingredients required for successful computations with density functional theory, it is useful to examine the performance of various exchange-correlation functionals; we do this here for 4s(N)3d(N') transition-metal atoms and their cations. We analyze the results using three ways to compute the energy of the open-shell states: the direct variational method, the weighted-averaged broken symmetry (WABS) method, and a new broken-symmetry method called the reinterpreted broken symmetry (RBS) method. We find the RBS method to be comparable in accuracy with the WABS method. By examining the overall accuracy in treating 18 multiplicity-changing excitations and 10 ionization potentials with the RBS method, 10 functionals are found to have a mean-unsigned error of systems, the M06-L functional is the most accurate. And by combining the results with our previous studies of p-block and 4d-series elements as well as databases for alkyl bond dissociation, main-group atomization energies, and π-π noncovalent interactions, we find five functionals, namely, PW6B95, MPW1B95, M08-SO, SOGGA11-X, and MPWB1K, to be highly recommended. We also studied the performance of PW86 and C09 exchange functionals, which have drawn wide interest in recent studies due to their claimed ability to reproduce Hartree-Fock exchange at long distance. By combining them with four correlation functionals, we find the performance of the resulting functionals disappointing both for 3d transition-metal chemistry and in broader tests, and thus we do not recommend PW86 and C09 as components of generalized

  6. The spin-unrestricted molecular Kohn-Sham solution and the analogue of Koopmans's theorem for open-shell molecules.

    Science.gov (United States)

    Gritsenko, O V; Baerends, E J

    2004-05-08

    -electron independent-particle model for interpretation and assignment of the experimental photoelectron spectra of open-shell molecules.

  7. Coupled cluster valence bond theory for open-shell systems with application to very long range strong correlation in a polycarbene dimer.

    Science.gov (United States)

    Small, David W; Head-Gordon, Martin

    2017-07-14

    The Coupled Cluster Valence Bond (CCVB) method, previously presented for closed-shell (CS) systems, is extended to open-shell (OS) systems. The theoretical development is based on embedding the basic OS CCVB wavefunction in a fictitious singlet super-system. This approach reveals that the OS CCVB amplitude equations are quite similar to those of CS CCVB, and thus that OS CCVB requires the same level of computational effort as CS CCVB, which is an inexpensive method. We present qualitatively correct CCVB potential energy curves for all low-lying spin states of P2 and Mn2(+). CCVB is successfully applied to the low-lying spin states of some model linear polycarbenes, systems that appear to be a hindrance to standard density functionals. We examine an octa-carbene dimer in a side-by-side orientation, which, in the monomer dissociation limit, exhibits maximal strong correlation over the length of the polycarbene.

  8. Measurement of ground state properties of neutron-rich nuclei on the r-process path between the N=50 and N=82 shells

    CERN Multimedia

    2007-01-01

    The evolution of the unknown ground-state ${\\beta}$-decay properties of the neutron-rich $^{84-89}$Ge, $^{90-93}$Se and $^{102-104}$Sr isotopes near the r-process path is of high interest for the study of the abundance peaks around the N=50 and N=82 neutron shells. At ISOLDE, beams of certain elements with sufficient isotopic purity are produced as molecular sidebands rather than atomic beams. This applies e.g, to germanium, separated as GeS$^{+}$, selenium separated as SeCO$^{+}$ and strontium separated as SrF$^{+}$. However, in case of neutron-rich isotopes produced in actinide targets, new "isobaric" background of atomic ions appears on the mass of the molecular sideband. For this particular case, the ECR charge breeder, positioned in the experimental hall after ISOLDE first mass separation, can be advantageously used as a purification device, by breaking the molecules and removing the molecular contaminants. This proposal indicates our interest in the study of basic nuclear structure properties of neutron...

  9. Light nuclei from chiral EFT interactions

    Science.gov (United States)

    Navrátil, P.; Gueorguiev, V. G.; Vary, J. P.; Ormand, W. E.; Nogga, A.; Quaglioni, S.

    2008-12-01

    Recent developments in nuclear theory allow us to make a connection between quantum chromodynamics (QCD) and low-energy nuclear physics. First, chiral effective field theory (χEFT) provides a natural hierarchy to define two-nucleon ( NN), three-nucleon ( NNN), and even four-nucleon interactions. Second, ab-initio methods have been developed capable to test these interactions for light nuclei. In this contribution, we discuss ab-initio no-core shell-model (NCSM) calculations for s-shell and p-shell nuclei with NN and NNN interactions derived within χEFT.

  10. Recent Advances in Shell Evolution with Shell-Model Calculations

    CERN Document Server

    Utsuno, Yutaka; Tsunoda, Yusuke; Shimizu, Noritaka; Honma, Michio; Togashi, Tomoaki; Mizusaki, Takahiro

    2014-01-01

    Shell evolution in exotic nuclei is investigated with large-scale shell-model calculations. After presenting that the central and tensor forces produce distinctive ways of shell evolution, we show several recent results: (i) evolution of single-particle-like levels in antimony and cupper isotopes, (ii) shape coexistence in nickel isotopes understood in terms of configuration-dependent shell structure, and (iii) prediction of the evolution of the recently established $N=34$ magic number towards smaller proton numbers. In any case, large-scale shell-model calculations play indispensable roles in describing the interplay between single-particle character and correlation.

  11. Origin of the increased open circuit voltage in PbS-CdS core-shell quantum dot solar cells

    NARCIS (Netherlands)

    Speirs, M. J.; Balazs, D. M.; Fang, H. -H.; Lai, L. -H.; Protesescu, L.; Kovalenko, M. V.; Loi, M. A.

    2015-01-01

    Lead sulfide quantum dots (PbS QDs) show great potential for efficient, low cost photovoltaic applications. Currently, device efficiencies are limited by the high density of trap states caused by lattice imperfections on the QD surface. Introducing a thin shell of a wide bandgap semiconductor to the

  12. Study of the influence of the shell correction energy on the nuclear reactions leading to the region of the superheavy nuclei; Etude de l'influence de l'energie de correction de couches sur les reactions nucleaires menant a la region des noyaux superlourds

    Energy Technology Data Exchange (ETDEWEB)

    Marchix, A

    2007-11-15

    The aim of this work is to study the influence of shell correction energy on the deexcitation of superheavy nuclei. For that purpose, a new statistical code, called Kewpie2, which is based on an original algorithm allowing to have access to very weak probabilities, was developed. The results obtained with Kewpie2 have been compared to the experimental data on residue cross sections obtained by cold fusion (Z=108 to Z=113) and by hot fusion (Z=112, Z=114 and Z=116), as well as data on fission times (Z=114, Z=120 and Z=126). Constraints on the microscopic structure of the studied nuclei have been obtained by means of the shell correction energy. By adjusting the intrinsic parameters of the models of fusion in order to reproduce the data on the fusion cross sections, this study shows the necessity of decreasing very strongly the shell correction energy predicted by the calculations of Moller and Nix, during the study of the residues cross sections as well for the nuclei produced by cold fusion as by hot fusion. On the other hand, during the confrontation of the results of Kewpie2 to the data on mean fission times, it is rather advisable to increase it. A shift of the proton shell closure predicted for Z=114 by the calculations of Moller and Nix towards larger Z would allow to explain these opposite conclusions. In this thesis, we also have shown the significant influence of the inclusion of isomeric states on fission times for the superheavy nuclei. (author)

  13. 跃层开洞楼板的剪力墙结构设计探讨%Shell Structure Analyzed of Floor Spring by Opening

    Institute of Scientific and Technical Information of China (English)

    郑炎彬

    2012-01-01

    The shell structure analyzed of floor spring by opening is represented in the building design, in order to discuss the effect of ab- normal structure to the max displacement in the floor, and some good points in the structure design.%本文通过介绍某高层跃层楼板开大洞的剪力墙结构计算分析,阐述了平面不规则结构对结构层间最大位移的影响,以及设计应该注意的若干要点。

  14. Excitation energies and properties of open-shell singlet molecules applications to a new class of molecules for nonlinear optics and singlet fission

    CERN Document Server

    Nakano, Masayoshi

    2014-01-01

    This brief investigates the diradical character, which is one of the ground-state chemical indices for 'bond weakness' or 'electron correlation' and which allows researchers to explore the origins of the electron-correlation-driven physico-chemical phenomena concerned with electronic, optical and magnetic properties as well as to control them in the broad fields of physics and chemistry. It then provides the theoretical fundamentals of ground and excited electronic structures of symmetric and asymmetric open-shell molecular systems by using model molecular systems. Moreover, it presents the th

  15. The emergence of deformation and rotational states in the many-nucleon quantum theory of nuclei

    Science.gov (United States)

    Rowe, D. J.

    2016-02-01

    The many-nucleon quantum mechanics of a nucleus is infinite-dimensional and, although simply defined, it has the potential for unlimited complexity. Nevertheless, the low-energy states of heavy open-shell nuclei exhibit properties that are remarkably well described by simple collective models. This paper examines this emergent simplicity from a perspective that closely parallels the emergence of shell structure in the Mayer-Jensen model. The result is an expression of the many-nucleon Hilbert space of a nucleus as an energy-ordered sum of subspaces each of which carries a microscopic version of the Bohr-Mottelson unified model. Each of the subspaces is characterized by nuclear states with a common intrinsic shape defined by its quadrupole moments. An emergence of simplicity and shape-coexistence in nuclei is then explained if it can be demonstrated that there is a relatively small and coherent mixing of the states of different collective subspaces.

  16. Shell effects in nuclear magnetization

    Energy Technology Data Exchange (ETDEWEB)

    Kondratyev, V.N.; Maruyama, Toshiki; Chiba, Satoshi [Advanced Science Research Center, Japan Atomic Energy Research Institute, Tokai, Ibaraki (Japan)

    2000-08-01

    The magnetization of nuclei in strong magnetic fields associated with magnetars' is considered within the shell model. It is demonstrated that the magnetic field gives rise to a phase-shift of the shell-oscillations in nuclear masses shifting significantly the nuclear magic numbers of the iron region towards smaller mass numbers. Shell-effects are found to result in anomalies of the nuclear magnetization. Such anomalies resemble the behavior associated with a phase transition. (author)

  17. Analytic first derivatives for a spin-adapted open-shell coupled cluster theory: Evaluation of first-order electrical properties

    Energy Technology Data Exchange (ETDEWEB)

    Datta, Dipayan, E-mail: datta@uni-mainz.de; Gauss, Jürgen, E-mail: gauss@uni-mainz.de [Institut für Physikalische Chemie, Johannes Gutenberg-Universität Mainz, Duesbergweg 10-14, D-55128 Mainz (Germany)

    2014-09-14

    An analytic scheme is presented for the evaluation of first derivatives of the energy for a unitary group based spin-adapted coupled cluster (CC) theory, namely, the combinatoric open-shell CC (COSCC) approach within the singles and doubles approximation. The widely used Lagrange multiplier approach is employed for the derivation of an analytical expression for the first derivative of the energy, which in combination with the well-established density-matrix formulation, is used for the computation of first-order electrical properties. Derivations of the spin-adapted lambda equations for determining the Lagrange multipliers and the expressions for the spin-free effective density matrices for the COSCC approach are presented. Orbital-relaxation effects due to the electric-field perturbation are treated via the Z-vector technique. We present calculations of the dipole moments for a number of doublet radicals in their ground states using restricted open-shell Hartree-Fock (ROHF) and quasi-restricted HF (QRHF) orbitals in order to demonstrate the applicability of our analytic scheme for computing energy derivatives. We also report calculations of the chlorine electric-field gradients and nuclear quadrupole-coupling constants for the CCl, CH{sub 2}Cl, ClO{sub 2}, and SiCl radicals.

  18. Basis set and electron correlation effects on the polarizability and second hyperpolarizability of model open-shell π-conjugated systems

    Science.gov (United States)

    Champagne, Benoı̂t; Botek, Edith; Nakano, Masayoshi; Nitta, Tomoshige; Yamaguchi, Kizashi

    2005-03-01

    The basis set and electron correlation effects on the static polarizability (α) and second hyperpolarizability (γ) are investigated ab initio for two model open-shell π-conjugated systems, the C5H7 radical and the C6H8 radical cation in their doublet state. Basis set investigations evidence that the linear and nonlinear responses of the radical cation necessitate the use of a less extended basis set than its neutral analog. Indeed, double-zeta-type basis sets supplemented by a set of d polarization functions but no diffuse functions already provide accurate (hyper)polarizabilities for C6H8 whereas diffuse functions are compulsory for C5H7, in particular, p diffuse functions. In addition to the 6-31G*+pd basis set, basis sets resulting from removing not necessary diffuse functions from the augmented correlation consistent polarized valence double zeta basis set have been shown to provide (hyper)polarizability values of similar quality as more extended basis sets such as augmented correlation consistent polarized valence triple zeta and doubly augmented correlation consistent polarized valence double zeta. Using the selected atomic basis sets, the (hyper)polarizabilities of these two model compounds are calculated at different levels of approximation in order to assess the impact of including electron correlation. As a function of the method of calculation antiparallel and parallel variations have been demonstrated for α and γ of the two model compounds, respectively. For the polarizability, the unrestricted Hartree-Fock and unrestricted second-order Møller-Plesset methods bracket the reference value obtained at the unrestricted coupled cluster singles and doubles with a perturbative inclusion of the triples level whereas the projected unrestricted second-order Møller-Plesset results are in much closer agreement with the unrestricted coupled cluster singles and doubles with a perturbative inclusion of the triples values than the projected unrestricted Hartree

  19. Dual origin of pairing in nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Idini, A. [University of Jyvaskyla, Department of Physics (Finland); Potel, G. [Michigan State University, National Superconducting Cyclotron Laboratory (United States); Barranco, F. [Escuela Superior de Ingenieros, Universidad de Sevilla, Departamento de Fìsica Aplicada III (Spain); Vigezzi, E., E-mail: enrico.vigezzi@mi.infn.it [INFN Sezione di Milano (Italy); Broglia, R. A. [Università di Milano, Dipartimento di Fisica (Italy)

    2016-11-15

    The pairing correlations of the nucleus {sup 120}Sn are calculated by solving the Nambu–Gor’kov equations, including medium polarization effects resulting from the interweaving of quasiparticles, spin and density vibrations, taking into account, within the framework of nuclear field theory (NFT), processes leading to self-energy and vertex corrections and to the induced pairing interaction. From these results one can not only demonstrate the inevitability of the dual origin of pairing in nuclei, but also extract information which can be used at profit to quantitatively disentangle the contributions to the pairing gap Δ arising from the bare and from the induced pairing interaction. The first is the strong {sup 1}S{sub 0} short-range NN potential resulting from meson exchange between nucleons moving in time reversal states within an energy range of hundreds of MeV from the Fermi energy. The second results from the exchange of vibrational modes between nucleons moving within few MeV from the Fermi energy. Short- (v{sub p}{sup bare}) and long-range (v{sub p}{sup ind}) pairing interactions contribute essentially equally to nuclear Cooper pair stability. That is to the breaking of gauge invariance in open-shell superfluid nuclei and thus to the order parameter, namely to the ground state expectation value of the pair creation operator. In other words, to the emergent property of generalized rigidity in gauge space, and associated rotational bands and Cooper pair tunneling between members of these bands.

  20. From heavy nuclei to super-heavy nuclei

    CERN Document Server

    Theisen, C

    2003-01-01

    The existence of super-heavy nuclei has been predicted nearly fifty years ago. Due to the strong coulomb repulsion, the stabilisation of these nuclei is possible only through shell effects. The reasons for this fragile stability, as well as the theoretical predictions concerning the position of the island of stability are presented in the first part of this lecture. In the second part, experiments and experimental techniques which have been used to synthesize or search for super-heavy elements are described. Spectroscopic studies performed in very heavy elements are presented in the following section. We close this lecture with techniques that are currently being developed in order to reach the superheavy island and to study the structure of very-heavy nuclei.

  1. Strange neutral currents in nuclei

    CERN Document Server

    Ressell, M T; Aufderheide, M B; Bloom, S D; Resler, D A

    1995-01-01

    We examine the effects on the nuclear neutral current Gamow-Teller (GT) strength of a finite contribution from a polarized strange quark sea. We perform nuclear shell model calculations of the neutral current GT strength for a number of nuclei likely to be present during stellar core collapse. We compare the GT strength when a finite strange quark contribution is included to the strength without such a contribution. As an example, the process of neutral current nuclear de-excitation via \

  2. Triaxial rotation in atomic nuclei

    Institute of Scientific and Technical Information of China (English)

    CHEN Yong-Shou; GAO Zao-Chun

    2009-01-01

    The Projected Shell Model has been developed to include the spontaneously broken axial symmetry so that the rapidly rotating triaxial nuclei can be described microscopically. The theory provides an useful tool to gain an insight into how a triaxial nucleus rotates, a fundamental question in nuclear structure. We shall address some current interests that are strongly associated with the triaxial rotation. A feasible method to explore the problem has been suggested.

  3. Studies of exotic light nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Cerny, J.

    1976-05-01

    For neutron-deficient nuclei, extension of the T/sub z/ = --3/2 series of strong beta-delayed proton precursors to /sup 61/Ge is discussed. For neutron-excess nuclei, heavy-ion induced, multi-nucleon transfer reaction studies of masses and energy levels of 2sld shell nuclei with T/sub z/ greater than or equal to 5/2 are covered. In addition, preliminary attempts to employ the (/sup 7/Li,/sup 2/He) reaction for the latter studies are shown; a new detection system capable of observing unbound final states as reaction products is demonstrated via investigations of the (..cap alpha..,/sup 2/He) reaction.

  4. Electric monopole transitions from low energy excitations in nuclei

    CERN Document Server

    Wood, J L; De Coster, C; Heyde, Kris L G

    1999-01-01

    Electric monopole (E0) properties are studied across the entire nuclear mass surface. Besides an introductory discussion of various model results (shell model, geometric vibrational and rotational models, algebraic models), we point out that many of the largest E0 transition strengths, $\\rho^2$(E0), are associated with shape mixing. We discuss in detail the manifestation of E0 transitions and present extensive data for~: single-closed shell nuclei, vibrational nuclei, well-deformed nuclei, nuclei that exhibit sudden ground-state changes, and nuclei that exhibit shape coexistence and intruder states. We also give attention to light nuclei, odd-A nuclei, and illustrate a suggested relation between $\\rho^2$(E0) and isotopic shifts.

  5. Global solutions of restricted open-shell Hartree-Fock theory from semidefinite programming with applications to strongly correlated quantum systems.

    Science.gov (United States)

    Veeraraghavan, Srikant; Mazziotti, David A

    2014-03-28

    We present a density matrix approach for computing global solutions of restricted open-shell Hartree-Fock theory, based on semidefinite programming (SDP), that gives upper and lower bounds on the Hartree-Fock energy of quantum systems. While wave function approaches to Hartree-Fock theory yield an upper bound to the Hartree-Fock energy, we derive a semidefinite relaxation of Hartree-Fock theory that yields a rigorous lower bound on the Hartree-Fock energy. We also develop an upper-bound algorithm in which Hartree-Fock theory is cast as a SDP with a nonconvex constraint on the rank of the matrix variable. Equality of the upper- and lower-bound energies guarantees that the computed solution is the globally optimal solution of Hartree-Fock theory. The work extends a previously presented method for closed-shell systems [S. Veeraraghavan and D. A. Mazziotti, Phys. Rev. A 89, 010502-R (2014)]. For strongly correlated systems the SDP approach provides an alternative to the locally optimized Hartree-Fock energies and densities with a certificate of global optimality. Applications are made to the potential energy curves of C2, CN, Cr2, and NO2.

  6. Global solutions of restricted open-shell Hartree-Fock theory from semidefinite programming with applications to strongly correlated quantum systems

    Energy Technology Data Exchange (ETDEWEB)

    Veeraraghavan, Srikant; Mazziotti, David A., E-mail: damazz@uchicago.edu [Department of Chemistry and The James Franck Institute, The University of Chicago, Chicago, Illinois 60637 (United States)

    2014-03-28

    We present a density matrix approach for computing global solutions of restricted open-shell Hartree-Fock theory, based on semidefinite programming (SDP), that gives upper and lower bounds on the Hartree-Fock energy of quantum systems. While wave function approaches to Hartree-Fock theory yield an upper bound to the Hartree-Fock energy, we derive a semidefinite relaxation of Hartree-Fock theory that yields a rigorous lower bound on the Hartree-Fock energy. We also develop an upper-bound algorithm in which Hartree-Fock theory is cast as a SDP with a nonconvex constraint on the rank of the matrix variable. Equality of the upper- and lower-bound energies guarantees that the computed solution is the globally optimal solution of Hartree-Fock theory. The work extends a previously presented method for closed-shell systems [S. Veeraraghavan and D. A. Mazziotti, Phys. Rev. A 89, 010502–R (2014)]. For strongly correlated systems the SDP approach provides an alternative to the locally optimized Hartree-Fock energies and densities with a certificate of global optimality. Applications are made to the potential energy curves of C{sub 2}, CN, Cr {sub 2}, and NO {sub 2}.

  7. 围壁补强的圆柱壳开孔结构有限元分析%Finite Element Analysis of Coaming Opening on the Cylindrical Shell

    Institute of Scientific and Technical Information of China (English)

    周猛猛; 杨宇华; 耿黎明; 刘朝骏

    2014-01-01

    The single radial opening is common on the pressure hull of submarine , and is stiffened by coaming usually .The ABAQUS software was utilized to calculate the stresses of cylindrical shell cut with single radial opening .The stress components were separated according to the equivalent principles to study the influence of coaming parameters upon stresses distribution , such as opening rate , thickness and height of coaming .%考虑到潜艇耐压壳上不可避免地要设置一些正交单圆孔,并采用围壁进行补强,利用ABAQUS通用有限元软件对该结构形式的系列模型进行求解,并利用等效原理分离出各应力成分,最终得出开孔率、围壁厚度、围壁高度以及围壁在壳体外的比例对各应力成分的影响规律。

  8. Realistic level density calculation for heavy nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Cerf, N. [Institut de Physique Nucleaire, Orsay (France); Pichon, B. [Observatoire de Paris, Meudon (France); Rayet, M.; Arnould, M. [Institut d`Astronomie et d`Astrophysique, Bruxelles (Belgium)

    1994-12-31

    A microscopic calculation of the level density is performed, based on a combinatorial evaluation using a realistic single-particle level scheme. This calculation relies on a fast Monte Carlo algorithm, allowing to consider heavy nuclei (i.e., large shell model spaces) which could not be treated previously in combinatorial approaches. An exhaustive comparison of the predicted neutron s-wave resonance spacings with experimental data for a wide range of nuclei is presented.

  9. Quark Degrees of Freedom in Finite Nuclei

    CERN Document Server

    Tsushima, K; Thomas, A W; Tsushima, Kazuo; Saito, Koichi; Thomas, Anthony W.

    1996-01-01

    Properties of finite nuclei are investigated based on relativistic Hartree equations which have been derived from a relativistic quark model of the structure of bound nucleons. Nucleons are assumed to interact through the (self-consistent) exchange of scalar ($\\sigma$) and vector ($\\omega$ and and the rms charge radius in $^{40}$Ca. Calculated properties of static, closed-shell nuclei, as well as symmetric nuclear matter are compared with experimental data and with the results of Quantum Hadrodynamics (QHD).

  10. Quantum Chemistry on Quantum Computers: A Polynomial-Time Quantum Algorithm for Constructing the Wave Functions of Open-Shell Molecules.

    Science.gov (United States)

    Sugisaki, Kenji; Yamamoto, Satoru; Nakazawa, Shigeaki; Toyota, Kazuo; Sato, Kazunobu; Shiomi, Daisuke; Takui, Takeji

    2016-08-18

    Quantum computers are capable to efficiently perform full configuration interaction (FCI) calculations of atoms and molecules by using the quantum phase estimation (QPE) algorithm. Because the success probability of the QPE depends on the overlap between approximate and exact wave functions, efficient methods to prepare accurate initial guess wave functions enough to have sufficiently large overlap with the exact ones are highly desired. Here, we propose a quantum algorithm to construct the wave function consisting of one configuration state function, which is suitable for the initial guess wave function in QPE-based FCI calculations of open-shell molecules, based on the addition theorem of angular momentum. The proposed quantum algorithm enables us to prepare the wave function consisting of an exponential number of Slater determinants only by a polynomial number of quantum operations.

  11. Reaching the cold regime: S(^1D) + H_2 and the Role of Long-Range Interactions in Open Shell Reactive Collisions

    CERN Document Server

    Lara, Manuel; Launay, J -M

    2010-01-01

    Reactive cross-sections for the collision of open shell S(^1D) atoms with ortho- and para-hydrogen, in the kinetic energy range 1-120 K, have been calculated using the hyperspherical quantum reactive scattering method developed by Launay et al. [Chem. Phys. Lett. 169, 473 (1990)]. Short-range interactions, described using the {\\em ab initio} potential energy surface by Ho et al. were complemented with an accurate description of the long-range interactions, where the main electrostatic (~R^{-5}) and dispersion (~ R^{-6}) contributions were considered. This allows the comparison with recent experimental measurements of rate constants and excitation functions for the title reaction at low temperatures [Berteloite et al., Phys. Rev. Lett., 2010]. The agreement is fairly good. The behavior in the considered energy range can be understood on the average in terms of a classical Langevin (capture) model, where the centrifugal barriers determine the amount of reactive flux which reaches the barrierless transition stat...

  12. Finite-field method with unbiased polarizable continuum model for evaluation of the second hyperpolarizability of an open-shell singlet molecule in solvents.

    Science.gov (United States)

    Inui, Tomoya; Shigeta, Yasuteru; Okuno, Katsuki; Baba, Takeshi; Kishi, Ryohei; Nakano, Masayoshi

    2013-10-15

    The static second hyperpolarizability γ of the complexes composed of open-shell singlet 1,3-dipole molecule involving a boron atom and a water molecule in aqueous phase are investigated by the finite-field (FF) method combined with a standard polarized continuum model (PCM) and with a newly proposed unbiased PCM (UBPCM). On the basis of the comparison with the results calculated by the FF method using the full quantum and the quantum-mechanical/molecular-mechanical and molecular-dynamics (QM/MM-MD) treatments, the present FF-UBPCM method is demonstrated to remedy the artificial overestimation of the γ caused by standard FF-PCM calculations and to well reproduce the FF-QM/MM-MD and FF-full-QM results with much lower costs.

  13. Resonances in s-d shell nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Schiffer, J.P.

    1981-01-01

    It appears that the system we have studied here, /sup 24/Mg(/sup 16/O,/sup 12/C)/sup 28/Si representing /sup 40/Ca as the composite nucleus, is perhaps the heaviest one that exhibits strong enough resonances that quantitative measurements may be contemplated. But we have uncovered only a small corner of what is there and even within this system a huge amount of work remains. The nature of these resonances is not yet clear. The sequence may perhaps have an explanation that is schematically outlined, namely that there are several families of quasistationary states in /sup 40/Ca, but that the slopes of these families do not necessarily coincide with the slope of the grazing partial waves that provide us with a narrow transparent strip of a window on the underlying structure of the nucleus. We must concentrate a lot of effort and ingenuity in order to maximize the information we gather through this window and only then may we hope to sensibly attempt forming hypotheses about the underlying simple pattern.

  14. Doubly magic properties in superheavy nuclei

    Institute of Scientific and Technical Information of China (English)

    HUANG Ya-Wei; ZHU Jian-Yu

    2009-01-01

    A systematic study of global properties of superheavy nuclei in the framework of the Liquid Drop Model and the Strutinsky shell correction method is performed. The evolution equilibrium deformations, TRS graphs and α-decay energies are calculated using the TRS model. The analysis covers a wide range of even-even superheavy nuclei from Z = 102 to 122. Magic numbers and their observable influence occurring in this region have been investigated. Shell closures appear at proton number Z = 114 and at neutron number N = 184.

  15. [Effect of acute hypoxia on the intensity of free radical processes in the basal nuclei of the brain, and the rat behaviour in the open field test under conditions of altered photoperiod].

    Science.gov (United States)

    Sopova, I Iu; Zamorskiĭ, I I

    2011-03-01

    The effect of acute hypoxia on the intensity of free radical processes in the basal nuclei (the nucleus caudatus, globus pallidus. nucleus accumbens. amygdaloid complex) of the brain, and the rat behaviour in the open field test has been studied under conditions of altered photoperiod. It has been shown that constant darkness levels the effect of acute hypoxia on the intensity of lipid peroxidation, preserves the activity of superoxide dismutase and catalase at a higher level, lowers the activity of glutathione peroxidase. Under light, the sensitivity of basal nuclei neurons to acute hypoxia is enhanced, the latter being reflected in intensification of lipid peroxidation at the expense of increased formation of dien conjugates. The activity of catalase at that considerably exceeds the level of even intact rats in all the structures. It has been established that an altered photoperiod modulates the effect of acute hypoxia on the parameters of rat's activity in the open field, the character of their change depending on the nature of a photophase change.

  16. Relativistic Multireference Many-body Perturbation Theory for Open-shell Ions with Multiple Valence Shell Electrons: the Transition Rates and Lifetimes of the Excited Levels in Chlorinelike Fe X

    Energy Technology Data Exchange (ETDEWEB)

    Ishikawa, Y; Santana, J A; Trabert, E

    2009-09-30

    A recently developed relatistic multireference many-body perturbation theory based on multireference configuration-interaction wavefunctions as zeroth order wavefunctions is outlined. The perturbation theory employs a general class of configuration-interaction wve functions as reference functions, and thus is applciable to multiple open valence shell systems with near degeneracy of a manifold of strongly interacting configurations. Multireference many-body perturbation calculations are reported for the ground and excited states of chlorine-like Fe X in which the near degeneracy of a manifold of strongly interacting configurations mandates a multireference treatment. Term energies of a total of 83 excited levels arising from the 3s{sup 2}3p{sup 5}, 3s3p{sup 6}, 3s{sup 2}3p{sup 4}3d, 3s3p{sup 5}3d, and 3s{sup 2}3p{sup 3}3d{sup 2} configurations of the ion are evaluated to high accuracy. Transition rates associated with E1/M1/E2/M2/E3 radiative decays and lifetimes of a number of excited levels are calculated and compared with laboratory measurements to critically evaluate recent experiments.

  17. Synthesis of superheavy nuclei with 238U target

    Institute of Scientific and Technical Information of China (English)

    2009-01-01

    The production of superheavy nuclei with Z=108-116 via hot fusion reactions of the neutron-rich projectiles with 238U target is systematically studied.The results show that the production cross sections of superheavy nuclei do not decrease monotonously as the atomic number Z increasing.The cross sections of the superheavy nuclei at Z = 112 and 115 are enhanced as compared with the whole Z-trend in synthesis of the superheavy nuclei,which clearly illustrates that the reactions with large negative Q-value and shell correction are more favorable to synthesize superheavy nuclei.

  18. Synthesis of superheavy nuclei with 238U target

    Institute of Scientific and Technical Information of China (English)

    LIU ZuHua; BAO JingDong

    2009-01-01

    The production of superheavy nuclei with Z=108-116 via hot fusion reactions of the neutron-rich projectiles with 238u target is systematically studied.The results show that the production cross sections of superheavy nuclei do not decrease monotonously as the atomic number Z increasing.The cross sections of the superheavy nuclei at Z=112 and 115 are enhanced as compared with the whole Z-trend in synthesis of the superheavy nuclei,which clearly illustrates that the reactions with large negative Q-value and shell correction are more favorable to synthesize superheavy nuclei.

  19. Study of neutron-rich nuclei structure around the N=28 shell closure using the in-beam gamma spectroscopy technique; Etude de la structure des noyaux riches en neutrons autour de la fermeture de couches N=28 par spectroscopie gamma en ligne

    Energy Technology Data Exchange (ETDEWEB)

    Bastin, B

    2007-10-15

    For a few years now, a loss of magicity in neutron-rich nuclei near the neutron drip-line at N=28 has been suggested and observed. Deformation in these nuclei has been observed. The deformation was explained in S isotopes as being due to a moderate reduction of the N=28 shell closure together with a proton induced collectivity originating from the near degeneracy of the proton d3/2 and s1/2 orbitals. As a consequence, the observed deformation seems to result from a subtle interplay between neutron and proton excitations. Since the proton configuration in the Si isotopes is expected to be more stable due to the Z=14 sub-shell gap, {sup 42}Si was considered as a key nucleus in order to distinguish the different effects responsible for the structural changes observed at N=28. Even if it is at the limits of our technical possibilities, an in-beam gamma-spectroscopy experiment using two-step fragmentation and one or several nucleons knockout reaction mechanisms was performed at GANIL. The measurement of the energy of the first excited state in {sup 42}Si, combined with the observation of {sup 38,40}Si and the spectroscopy of {sup 41,43}P, has given evidence for the loss of magicity at N=28 far from stability. Modifications of the effective interaction used in modern shell model calculations have been completed following this investigation, increasing its predictive character. This study confirms the role of the tensor force and the density dependence of the spin-orbit interaction in the collapse of the N=28 shell closure. (author)

  20. Multiphonon giant resonances in nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Aumann, T. [Mainz Univ. (Germany). Inst. fuer Kernchemie; Bortignon, P.F. [Milan Univ. (Italy). Dipt. di Fisica]|[Istituto Nazionale di Fisica Nucleare, Milan (Italy); Emling, H. [Gesellschaft fuer Schwerionenforschung mbH, Darmstadt (Germany)

    1998-07-01

    We review the present knowledge of multiphonon giant resonances in nuclei. Theoretical concepts approaching the intrinsic structure and excitation mechanisms of multi-phonon states are discussed. The available experimental results are summarized, including a brief description of applied techniques. This review emphasizes electromagnetic excitations of double dipole resonances. Open questions and possible routes toward a solution are addressed. (orig.)

  1. Reaction cross section measurements of neutron-rich exotic nuclei in the vicinity of closed shells N=20 and N=28; Mesures de section efficace de reaction de noyaux exotiques riches en neutrons dans la zone de fermeture des couches N=20 et N=28

    Energy Technology Data Exchange (ETDEWEB)

    Khouaja, A

    2003-12-01

    Using the direct method, the mean energy integrated reaction cross section was investigated for a wide range of neutron-rich nuclei (N {yields} Ar) at GANIL. Using the parametrisation of S. Kox, 19 new radii measurements (reaction cross sections) were obtained. By the isotopic, isotonic and isospin dependence, the evolution of the strong reduced radius was studied according to the excess of neutrons. New halo effect is proposed to the nuclei of Mg{sup 35} and S{sup 44}. A quadratic parametrization is also proposed for the nuclear radius as a function of the isospin in the region of closed shells N=8 and N=28. In addition, we used a modified version of the Glauber model for studying the tail and matter distribution of nuclei. Indeed, using our new data the effects of the nuclear size (root mean square radii) and the matter distribution (diffusivity) were de-convoluted for each isotope. The root mean square radii of Na and Mg isotopes obtained so far were consistent with the ones from literature. (author)

  2. Surface-initiated ring-opening metathesis polymerization (SI-ROMP) to attach a tethered organic corona onto CdSe/ZnS core/shell quantum dots

    Science.gov (United States)

    Vatansever, Fatma; Hamblin, Michael R.

    2016-10-01

    Core-shell CdSe/ZnS quantum dots (QDs) are useful as tunable photostable fluorophores for multiple applications in industry, biology, and medicine. However, to achieve the optimum optical properties, the surface of the QDs must be passivated to remove charged sites that might bind extraneous substances and allow aggregation. Here we describe a method of growing an organic polymer corona onto the QD surface using the bottom-up approach of surface-initiated ring-opening metathesis polymerization (SI-ROMP) with Grubbs catalyst. CdSe/ZnS QDs were first coated with mercaptopropionic acid by displacing the original tri-octylphosphine oxide layer, and then reacted with 7-octenyl dimethyl chlorosilane. The resulting octenyl double bonds allowed the attachment of ruthenium alkylidene groups as a catalyst. A subsequent metathesis reaction with strained bicyclic monomers (norbornene-dicarbonyl chloride (NDC), and a mixture of NDC and norbornenylethylisobutyl-polyhedral oligomeric silsesquioxane (norbornoPOSS)) allowed the construction of tethered organic homo-polymer or co-polymer layers onto the QD. Compounds were characterized by FT-IR, 1H-NMR, X-ray photoelectron spectroscopy, differential scanning calorimetry, and transmission electron microscopy. Atomic force microscopy showed that the coated QDs were separate and non-aggregated with a range of diameter of 48-53 nm.

  3. Exchange effects in elastic collisions of spin-polarized electrons with open-shell molecules with $^3\\Sigma_g^-$ symmetry

    CERN Document Server

    Tashiro, Motomichi

    2007-01-01

    The spin-exchange effect in spin-polarized electron collisions with unpolarized open-shell molecules, O$_2$, B$_2$, S$_2$ and Si$_2$, has been studied by the R-matrix method with the fixed-bond approximation. All of these molecules have ${}^3 \\Sigma_{g}^{-}$ symmetry in their ground states. Usual integrated cross sections with unpolarized electrons has also been studied. We used the complete active space self consistent field orbitals and put more than 10 target electronic states in the R-matrix models. In electron O$_2$ elastic collisions, calculated polarization fractions agree well with the experimental results, especially around the ${}^4 \\Sigma_u^-$ resonance. In e-B$_2$, S$_2$ and Si$_2$ elastic collisions, larger spin-exchange effect is observed compared to the e-O$_2$ elastic collisions. In all four cases, spin-exchange effect becomes prominent near resonances. This association of resonance and magnitude of the spin-exchange effect was studied by explicitly removing the resonance configurations from t...

  4. Quantum master equation method based on the broken-symmetry time-dependent density functional theory: application to dynamic polarizability of open-shell molecular systems.

    Science.gov (United States)

    Kishi, Ryohei; Nakano, Masayoshi

    2011-04-21

    A novel method for the calculation of the dynamic polarizability (α) of open-shell molecular systems is developed based on the quantum master equation combined with the broken-symmetry (BS) time-dependent density functional theory within the Tamm-Dancoff approximation, referred to as the BS-DFTQME method. We investigate the dynamic α density distribution obtained from BS-DFTQME calculations in order to analyze the spatial contributions of electrons to the field-induced polarization and clarify the contributions of the frontier orbital pair to α and its density. To demonstrate the performance of this method, we examine the real part of dynamic α of singlet 1,3-dipole systems having a variety of diradical characters (y). The frequency dispersion of α, in particular in the resonant region, is shown to strongly depend on the exchange-correlation functional as well as on the diradical character. Under sufficiently off-resonant condition, the dynamic α is found to decrease with increasing y and/or the fraction of Hartree-Fock exchange in the exchange-correlation functional, which enhances the spin polarization, due to the decrease in the delocalization effects of π-diradical electrons in the frontier orbital pair. The BS-DFTQME method with the BHandHLYP exchange-correlation functional also turns out to semiquantitatively reproduce the α spectra calculated by a strongly correlated ab initio molecular orbital method, i.e., the spin-unrestricted coupled-cluster singles and doubles.

  5. Translationally invariant treatment of pair correlations in nuclei; 1, spin and isospin dependent correlations

    CERN Document Server

    Guardiola, R; Navarro, J; Bishop, R F; Puente, A; Walet, N R; Walet, Niels R.

    1996-01-01

    We study the extension of our translationally invariant treatment of few-body nuclear systems to heavier nuclei. At the same time we also introduce state-dependent correlation operators. Our techniques are tailored to those nuclei that can be dealt with in $LS$ coupling, which includes all nuclei up to the shell closure at $A=40$. We study mainly $p$-shell nuclei in this paper. A detailed comparison with other microscopic many-body approaches is made, using a variety of schematic nuclear interactions. It is shown that our methodology produces very good energies, and presumably also wave functions, for medium mass nuclei.

  6. Analytic view at alpha clustering in even-even heavy nuclei near magic numbers 82 and 126

    Energy Technology Data Exchange (ETDEWEB)

    Ahmed, Saad M.S. [Universiti Kebangsaan Malaysia, School of Applied Physics, Faculty of Science and Technology, Selangor (Malaysia); University of Malaya, Department of Physics, Faculty of Science, Kuala Lumpur (Malaysia); University of Malaya, Quantum Science Centre, Department of Physics, Faculty of Science, Kuala Lumpur (Malaysia); Yahaya, Redzuwan; Radiman, Shahidan; Yasir, Muhamad Samudi [Universiti Kebangsaan Malaysia, School of Applied Physics, Faculty of Science and Technology, Selangor (Malaysia); Kassim, Hasan Abu; Khandaker, Mayeen Uddin [University of Malaya, Department of Physics, Faculty of Science, Kuala Lumpur (Malaysia); University of Malaya, Quantum Science Centre, Department of Physics, Faculty of Science, Kuala Lumpur (Malaysia)

    2015-02-01

    Most studies on the determination of the alpha-decay preformation factor have used decay formulae. The preformation factor is known to contain abundant information on the nuclear structure. The successful determination of the preformation factor through the cluster formation model (CFM) motivates this study to determine the factor for nuclei near the magic numbers and present results in an analytic study based on different comparisons and observations. The difference between preformation factors obtained from CFM and from the decay formula method is significant. The formula method is used for the entire process of alpha decay as a transition between two states, whereas CFM is applied for the initial state of alpha formation. The preformation factor obtained using CFM and clusterization state representation was first compared with that obtained from the decay formula. Results were used to investigate alpha formation in even-even heavy nuclei, including 72 < Z < 92 and 92 < N < 142, near the magic numbers Z = 82 and N = 126. The values of the preformation factor were discussed and explained in detail according to the clusterization state representation to describe the most possible states of ground-state nuclei. The alpha clustering described through CFM is found to be consistent with that described using the decay formula for the open-shell nuclei of N < 126. The presence of more nucleons in the open-shell nuclei results in lower probability for alpha clustering and lower value of the preformation factor. However, few nucleons beyond the closed shell can cause higher probability for alpha clustering and larger value of the preformation factor. The maximum and minimum of the alpha-cluster formation occur in the nucleus of the double-shell closure (with N = 126 and Z = 82) and in the nucleus of two protons and two neutrons more. This formation probability is sensitive to the subshells, leading to the possibility of more clusterization states, including core

  7. A Hirshfeld interpretation of the charge, spin distribution, and polarity of the dipole moment of the open shell (3Sigma-) nitrogen halides: NF, NCl, and NBr.

    Science.gov (United States)

    Harrison, James F

    2009-07-28

    We calculated the dipole moment function for the ground (3)Sigma(-)(m(S) = +1) state of the open shell molecules, NF, NCl, and NBr, and analyzed it in terms of the charge and spin distribution and the induced atomic dipoles using the Hirshfeld partitioning of the electron density. The smallest dipole moment (0.026ea(0)) obtains with NF, in which the atoms have the largest difference in electronegativity, while the dipole moments in NCl and NBr are 0.441ea(0) and 0.506ea(0), respectively. All dipoles have the N(-)X(+) polarity. In the sigma system alpha spin electrons flow from N to the halogen while beta spin electrons flow in the opposite direction and interestingly from both the sigma and the pi systems of the halogen to the sigma system of N. In NF the number of beta spins lost by F is essentially equal to the number of alpha spins gained and the atomic charges are essentially 0. The small dipole in NF is the result of a slight imbalance in the induced atomic dipoles. For NCl and NBr the halogen loses more beta spins than it gains alpha spins resulting in the polarity N(-)X(+). It is interesting that at equilibrium N gained electrons in the pi system while the halogen lost pi electrons relative to the separated atoms. This however is not back donation in the usual sense because the electrons gained by N have alpha spin while those lost by the halogen have beta spin. Detailed examination of the spin flow shows that the excess alpha electrons in the pi system of N come from an intra-atomic transfer from the N sigma system. The induced atomic dipole moments essentially cancel at all internuclear separations and the polarity of the dipole moment accurately reflects the molecular charge distribution.

  8. Evidence for {open_quotes}magnetic rotation{close_quotes} in nuclei: New results on the M1-bands of {sup 198,199}Pb

    Energy Technology Data Exchange (ETDEWEB)

    Clark, R.M. [Lawrence Berkeley National Lab., CA (United States)

    1996-12-31

    Lifetimes of states in four of the M1-bands in {sup 198,199}Pb have been determined through a Doppler Shift Attenuation Method measurement performed using the Gammasphere array. The deduced B(M1) values, which are a sensitive probe of the underlying mechanism for generating these sequences, show remarkable agreement with Tilted Axis Cranking (TAC) calculations. Evidence is also presented for the possible termination of the bands. The results represent clear evidence for a new concept in nuclear excitations: {open_quote}magnetic rotation{close_quote}.

  9. Shell Model Study on the Proton Pigmy Dipole Resonances in ~(17, 18)Ne

    Institute of Scientific and Technical Information of China (English)

    2011-01-01

    The proton pygmy dipole resonances (PDRs) in proton rich nuclei 17, 18Ne have been investigated in the framework of interacting shell model. The shell model with the self-consistent Skyrme-Hartree-Fock wave functions has well reproduced

  10. Fission and Properties of Neutron-Rich Nuclei

    Science.gov (United States)

    Hamilton, Joseph H.; Ramayya, A. V.; Carter, H. K.

    2008-08-01

    Opening session. Nuclear processes in stellar explosions / M. Wiescher. In-beam [symbol]-ray spectroscopy of neutron-rich nuclei at NSCL / A. Gade -- Nuclear structure I. Shell-model structure of neutron-rich nuclei beyond [symbol]Sn / A. Covello ... [et al.]. Shell structure and evolution of collectivity in nuclei above the [symbol]Sn core / S. Sarkar and M. S. Sarkar. Heavy-ion fusion using density-constrained TDHF / A. S. Umar and V. E. Oberacker. Towards an extended microscopic theory for upper-fp shell nuclei / K. P. Drumev. Properties of the Zr and Pb isotopes near the drip-line / V. N. Tarasov ... [et al.]. Identification of high spin states in [symbol] Cs nuclei and shell model calculations / K. Li ... [et al.]. Recent measurements of spherical and deformed isomers using the Lohengrin fission-fragment spectrometer / G. S. Simpson ... [et al.] -- Nuclear structure II. Nuclear structure investigation with rare isotope spectroscopic investigations at GSI / P. Boutachkov. Exploring the evolution of the shell structures by means of deep inelastic reactions / G. de Anaelis. Probing shell closures in neutron-rich nuclei / R. Krücken for the S277 and REX-ISOLDEMINIBALL collaborations. Structure of Fe isotopes at the limits of the pf-shell / N. Hoteling ... [et al.]. Spectroscopy of K isomers in shell-stabilized trans-fermium nuclei / S. K. Tandel ... [et al.] -- Radioactive ion beam facilities. SPIRAL2 at GANIL: a world leading ISOL facility for the next decade / S. Gales. New physics at the International Facility for Antiproton and Ion Research (FAIR) next to GSI / I. Augustin ... [et al.]. Radioactive beams from a high powered ISOL system / A. C. Shotter. RlKEN RT beam factory / T. Motobayashi. NSCL - ongoing activities and future perspectives / C. K. Gelbke. Rare isotope beams at Argonne / W. F. Henning. HRIBF: scientific highlights and future prospects / J. R. Beene. Radioactive ion beam research done in Dubna / G. M. Ter-Akopian ... [et al.] -- Fission I

  11. Relativistic continuum random phase approximation in spherical nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Daoutidis, Ioannis

    2009-10-01

    Covariant density functional theory is used to analyze the nuclear response in the external multipole fields. The investigations are based on modern functionals with zero range and density dependent coupling constants. After a self-consistent solution of the Relativistic Mean Field (RMF) equations for the nuclear ground states multipole giant resonances are studied within the Relativistic Random Phase Approximation (RRPA), the small amplitude limit of the time-dependent RMF. The coupling to the continuum is treated precisely by calculating the single particle Greens-function of the corresponding Dirac equation. In conventional methods based on a discretization of the continuum this was not possible. The residual interaction is derived from the same RMF Lagrangian. This guarantees current conservation and a precise decoupling of the Goldstone modes. For nuclei with open shells pairing correlations are taken into account in the framework of BCS theory and relativistic quasiparticle RPA. Continuum RPA (CRPA) presents a robust method connected with an astonishing reduction of the numerical effort as compared to conventional methods. Modes of various multipolarities and isospin are investigated, in particular also the newly discovered Pygmy modes in the vicinity of the neutron evaporation threshold. The results are compared with conventional discrete RPA calculations as well as with experimental data. We find that the full treatment of the continuum is essential for light nuclei and the study of resonances in the neighborhood of the threshold. (orig.)

  12. Study of the N=28 shell closure by one neutron transfer reaction: astrophysical application and {beta}-{gamma} spectroscopy of neutron rich nuclei around N=32/34 and N=40; Etude de la fermeture de couche N=28 autour du noyau {sub 18}{sup 46}Ar{sub 28} par reaction de transfert d'un neutron: application a l'astrophysique et Spectroscopie {beta}-{gamma} de noyaux riches en neutrons de N=32/34 et N=40

    Energy Technology Data Exchange (ETDEWEB)

    Gaudefroy, L

    2005-09-15

    The study of the N=28 shell closure has been presented as well as its astrophysical implications. Moreover the structure of neutron rich nuclei around N=32/34 and 40 was studied. The N=28 shell closure has been studied trough the one neutron transfer reaction on {sup 44,46}Ar nuclei. Excitation energies of states in {sup 45,47}Ar nuclei have been obtained, as well as their angular momenta and spectroscopic factors. These results were used to show that N=28 is still a good magic number in the argon isotopic chain. We interpreted the evolution of the spin-orbit partner gaps in terms of the tensor monopolar proton-neutron interaction. Thanks to this latter, we showed it is not necessary to summon up a reduction of the intensity of the spin-orbit force in order to explain this evolution in N=29 isotopes from calcium to argon chains. The neutron capture rates on {sup 44,46}Ar have been determined thanks to the results of the transfer reaction. Their influence on the nucleosynthesis of {sup 46,48}Ca was studied. We proposed stellar conditions to account for the abnormal isotopic ratio observed in the Allende meteorite concerning {sup 46,48}Ca isotopes. The beta decay and gamma spectroscopy of neutron rich nuclei in the scandium to cobalt region has been studied. We showed that beta decay process is dominated by the {nu}f{sub 5/2} {yields} {pi}f{sub 7/2} Gamow-Teller transition. Moreover, we demonstrated that the {nu}g{sub 9/2} hinders this process in the studied nuclei, and influences their structure, by implying the existence of isomers. Our results show that N=34 is not a magic number in the titanium chain and the superior ones. (author)

  13. Spherical nuclei near the stability line and far from it

    Energy Technology Data Exchange (ETDEWEB)

    Isakov, V. I., E-mail: visakov@thd.pnpi.spb.ru [National Research Centre Kurchatov Institute, Petersburg Nuclear Physics Institute (Russian Federation)

    2016-11-15

    Results of microscopic and semiphenomenological calculations of features of spherical nuclei lying near the stability line and far from it are presented. The reason why the nuclei being considered are spherical is that they are magic at least in one nucleon sort. The present analysis is performed for Z = 50 and Z = 28 isotopes and for N = 50 isotones, the region extending from neutron-rich to neutron-deficient nuclei being covered. The isotopic dependence of the mean-field spin–orbit nuclear potential is revealed; systematics of energies of levels and probabilities for electromagnetic transitions is examined; and root-mean-square radii of nuclei are calculated, along with the proton- and neutron-density distributions in them. Nuclei in the vicinity of closed shells are considered in detail, and the axial-vector weak coupling constant in nuclei is evaluated. A systematic comparison of the results of calculations with experimental data is performed.

  14. Alpha decay chains from superheavy nuclei

    CERN Document Server

    Samanta, C

    2008-01-01

    Magic islands for extra-stable nuclei in the midst of the sea of fission-instability were predicted to be around Z=114, 124 or, 126 with N=184, and Z=120, with N=172. Whether these fission-survived superheavy nuclei with high Z and N would live long enough for detection or, undergo alpha-decay in a very short time remains an open question. Alpha-decay half lives of nuclei with 130 118 are found to have alpha-decay half lives of the order of microseconds or, less.

  15. Survey of Excited State Neutron Spectroscopic Factors for Z=8-28 Nuclei

    Science.gov (United States)

    Tsang, M. B.; Lee, Jenny; Su, S. C.; Dai, J. Y.; Horoi, M.; Liu, H.; Lynch, W. G.; Warren, S.

    2009-02-01

    We have extracted 565 neutron spectroscopic factors of sd and fp shell nuclei by systematically analyzing more than 2000 measured (d, p) angular distributions. We are able to compare 125 of the extracted spectroscopic factors to values predicted by large-basis shell-model calculations and evaluate the accuracies of spectroscopic factors predicted by different shell-model interactions in these regions. We find that the spectroscopic factors predicted for most excited states of sd-shell nuclei using the latest USDA or USDB interactions agree with the experimental values. For fp shell nuclei, the inability of the current models to account for the core excitation and fragmentation of the states leads to considerable discrepancies. In particular, the agreement between data and shell-model predictions for Ni isotopes is not better than a factor of 2 using either the GXPF1A or the XT interaction.

  16. Collective excitations in nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Chomaz, Ph. [Grand Accelerateur National d`Ions Lourds (GANIL), 14 - Caen (France); Collaboration: La Direction des Sciences de la Matiere du CEA (FR); Le Fonds National de la Recherche Scientifique de Belgique (BE)

    1998-12-31

    The properties of the nucleus cannot be reduced to the properties of its constituents: it is a complex system. The fact that many properties of the nucleus are consequences of the existence of mean-field potential is a manifestation of this complexity. In particular, the nucleons can thus self-organize in collective motions such as giant resonances. Therefore the study of this collective motions is a very good tool to understand the properties of the nucleus itself. The purpose of this article is to stress some aspects of these collective vibrations. We have studied how an ensemble of fermions as the nucleus can self-organize in collective vibrations which are behaving like a gas of bosons in weak interaction. Understanding of these phenomena remains one of the important subjects of actuality in the context of quantal systems in strong interaction. In particular, the study of the states with one or two vibration quanta provides a direct information on the structure of nuclei close to their ground states. Moreover, some collective states appear to be very robust against the onset of chaos. This is the case of the hot giant dipole built on top of a hot nucleus which seems to survive up to rather high temperatures. Their sudden disappearance is still a subject of controversy. It may be that the mean-field and the associated collective states are playing a crucial role also in catastrophic processes such as the phase-transitions. Indeed, when the system is diluted the collective vibrations may become unstable and it seems that these unstable modes provide a natural explanation to the self organization of the system in drops. Finally, considering the diversity of the different structures of exotic nuclei one may expect new vibration types. All these studies are showing the diversity of the collective motions of strongly correlated quantum systems such as the nucleus but many open questions remain to be solved. (authors) 304 refs., 53 figs., 5 tabs.

  17. Nucleon localization in light and heavy nuclei

    CERN Document Server

    Zhang, C L; Nazarewicz, W

    2016-01-01

    An electron localization measure was originally introduced to characterize chemical bond structures in molecules. Recently, a nucleon localization based on Hartree-Fock densities has been introduced to investigate $\\alpha$-cluster structures in light nuclei. Compared to the local nucleonic densities, the nucleon localization function has been shown to be an excellent indicator of shell effects and cluster correlations. Using the spatial nucleon localization measure, we investigate the cluster structures in deformed light nuclei and study the emergence of fragments in fissioning heavy nuclei. To illustrate basic concepts of nucleon localization, we employ the deformed harmonic oscillator model. Realistic calculations are carried out using self-consistent nuclear density functional theory with quantified energy density functionals optimized for fission studies. We study particle densities and spatial nucleon localization distributions for deformed cluster configurations of $^{8}$Be and $^{20}$Ne, and also along...

  18. Synthesis of superheavy nuclei: Obstacles and opportunities

    Directory of Open Access Journals (Sweden)

    Zagrebaev V.I.

    2015-01-01

    Full Text Available There are only 3 methods for the production of heavy and superheavy (SH nuclei, namely, fusion reactions, a sequence of neutron capture and beta(- decay and multinucleon transfer reactions. Low values of the fusion cross sections and very short half-lives of nuclei with Z<120 put obstacles in synthesis of new elements. At the same time, an important area of SH isotopes located between those produced in the cold and hot fusion reactions remains unstudied yet. This gap could be filled in fusion reactions of 48Ca with available lighter isotopes of Pu, Am, and Cm. New neutron-enriched isotopes of SH elements may be produced with the use of a 48Ca beam if a 250Cm target would be prepared. In this case we get a real chance to reach the island of stability owing to a possible beta(+ decay of 291114 and 287112 nuclei formed in this reaction with a cross section of about 0.8 pb. A macroscopic amount of the long-living SH nuclei located at the island of stability may be produced by using the pulsed nuclear reactors of the next generation only if the neutron fluence per pulse will be increased by about three orders of magnitude. Multinucleon transfer processes look quite promising for the production and study of neutron-rich heavy nuclei located in upper part of the nuclear map not reachable by other reaction mechanisms. Reactions with actinide beams and targets are of special interest for synthesis of new neutron-enriched transfermium nuclei and not-yet-known nuclei with closed neutron shell N=126 having the largest impact on the astrophysical r-process. The estimated cross sections for the production of these nuclei allows one to plan such experiments at currently available accelerators.

  19. Effect of Baffle Opening on the Performance of Shell-and-T ube Heat Exchanger%折流板开孔对管壳式换热器性能的影响

    Institute of Scientific and Technical Information of China (English)

    郭土; 马贵阳; 石龙; 黄腾龙

    2013-01-01

    The traditional baffle heat exchanger is widely used for its simple structure ,safety and reliability and adaptability advantages ,but the traditional baffle heat exchanger has many weaknesses :its thermal efficiency is low ,shell side pressure loss is bigger and easy scaling .It is a very important engineering significance through improving the vertical baffles'structure to ameliorate the shell and tube heat exchanger's flow and heat transfer condition of shell side and reduce its energy dissipation . Baffle opening to improve the structure of a gap 0 .2D height was studied by numerical simulation method .The velocity field and temperature field numerically simulated ordinary baffles heat exchanger and baffle opening heat exchanger . Under the condition of the same entering velocity of shell side ,the thermal effect of baffle opening heat exchanger is better than ordinary vertical baffle plate heat exchanger .And when the entering velocity of shell side is slow ,the effect is better .%传统的弓形折流板换热器因其结构简单、安全可靠及适应性强等优点应用非常广泛,但是传统的弓形折流板换热器换热效率较低,壳程压力损失较大,容易结垢。因此,通过对弓形折流板结构进行改进以改善管壳式换热器的壳程流动传热状况,减小其能耗损失具有十分重大的工程意义。采用数值模拟的方法,对缺口高度为0.2D的折流板进行开孔优化研究,对不同壳程进口流速下的普通弓形折流板换热器和折流板开孔换热器的壳程流场及温度场分别进行了数值模拟。在壳程进口流速相等的条件下,折流板开孔的换热器比普通弓形折流板换热器的换热效果好;壳程进口速度较低时,效果最明显。

  20. Inclusive quasielastic scattering of polarized electrons from polarized nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Amaro, J.E. [Massachusetts Inst. of Tech., Cambridge, MA (United States). Center for Theoretical Physics]|[Universidad de Granada (Spain). Dept. de Fisica Moderna]|[Massachusetts Inst. of Tech., Cambridge, MA (United States). Lab. for Nuclear Science]|[Massachusetts Inst. of Tech., Cambridge, MA (United States). Dept. of Physics; Caballero, J.A. [Consejo Superior de Investigaciones Cientificas (CSIC), Madrid (Spain). Inst. de Estructura de la Materia]|[Sevilla Univ. (Spain). Dept. de Fisica Atomica, Molecular y Nuclear; Donnelly, T.W. [Massachusetts Inst. of Tech., Cambridge, MA (United States). Center for Theoretical Physics]|[Massachusetts Inst. of Tech., Cambridge, MA (United States). Lab. for Nuclear Science]|[Massachusetts Inst. of Tech., Cambridge, MA (United States). Dept. of Physics; Moya de Guerra, E. [Consejo Superior de Investigaciones Cientificas (CSIC), Madrid (Spain). Inst. de Estructura de la Materia

    1996-12-23

    The inclusive quasielastic response functions that appear in the scattering of polarized electrons from polarized nuclei are computed and analyzed for several closed-shell-minus-one nuclei with special attention paid to {sup 39}K. Results are presented using two models for the ejected nucleon - when described by a distorted wave in the continuum shell model or by a plane wave in PWIA with on- and off-shell nucleons. Relativistic effects in kinematics and in the electromagnetic current have been incorporated throughout. Specifically, the recently obtained expansion of the electromagnetic current in powers only of the struck nucleon`s momentum is employed for the on-shell current and the effects of the first-order terms (spin-orbit and convection) are compared with the zeroth-order (charge and magnetization) contributions. The use of polarized inclusive quasielastic electron scattering as a tool for determining near-valence nucleon momentum distributions is discussed. (orig.).

  1. Dielectronic Recombination In Active Galactic Nuclei

    Science.gov (United States)

    Lukić, D.; Savin, D. W.; Schnell, M.; Brandau, C.; Schmidt, E.; Schippers, S.; Müller, A.; Lestinsky, M.; Sprenger, F.; Wolf, A.; Altun, Z.; Badnell, N. R.

    2006-05-01

    Recent X-ray satelitte observations of active galactic nuclei point out shortcomings in our understanding of low temperature dielectronic recombination (DR) for iron M- shell ions. In order to resolve this issue and to provide reliable iron M-shell DR data for modeling astrophysical plasmas, we are carrying out a series of laboratory measurements using the heavy-ion Test Storage Ring at the Max- Plank-Institute for Nuclear Physics in Heidelberg, Germany. Storage rings are currently the only laboratory method capable of studying low temperature DR. We use our results to produce experimentally- derived DR rate coefficients. We are also providing our data to atomic theorist to benchmark their DR calculations. Here we will report our recent DR results for selected Fe M-shell ions. At temperatures where these ions are predicted to form in photoionized gas, we find a significant discrepancy between our experimental results and previously recommended DR rate coefficients.

  2. Nucleon pairing correlations and the α cluster preformation probability inside heavy and superheavy nuclei

    Science.gov (United States)

    Seif, W. M.

    2015-01-01

    The presence of paired or unpaired protons and neutrons in the open-shell radioactive α emitter affects the preformation probability of the α cluster inside it. The α-preformation probability inside the odd ( Z )-even ( N ) , even ( Z )-odd ( N ) , and odd ( Z )-odd ( N ) α emitters is investigated. The study is restricted to those decays with no angular momentum transfer to make a precise prediction about the mere pairing effect. The extended cluster model of α decay and the WKB approximation are used by taking into account the deformation degrees of freedom to carry out the calculations for 105 parent nuclei in the mass region of A =175 -289 . The α + daughter interaction potential is calculated by using the Hamiltonian energy-density approach in terms of the SLy4 Skyrme-like interaction, then it is implemented to find the average decay width over the different orientations. The half-life of the decay is then estimated and employed in turn to extract the α-preformation probability by taking account of errors on both the released energy and the experimental half-life time. According to the present calculations, it is found that the α cluster preformation probability inside the nuclei which have unpaired nucleons is less than it would be in the neighboring nuclei of the same shell and subshell closures but have no unpaired nucleons. In particular, the effect of the single unpaired neutron in the even ( Z )-odd ( N ) nuclei is slightly larger than that of the single unpaired proton in the odd ( Z )-even ( N ) ones. The effect of the unpaired nucleons appears more clearly in the odd ( Z )-odd ( N ) nuclei which have both an unpaired neutron and an unpaired proton. Based on the obtained results, an empirical pairing term is added to the empirical formula [J. Phys. G 40, 105102 (2013), 10.1088/0954-3899/40/10/105102] that relates the α cluster preformation probability to the proton and neutron numbers outside the closed shells of the parent nucleus.

  3. Dynamic Analysis of Shells

    Directory of Open Access Journals (Sweden)

    Charles R. Steele

    1995-01-01

    Full Text Available Shell structures are indispensable in virtually every industry. However, in the design, analysis, fabrication, and maintenance of such structures, there are many pitfalls leading to various forms of disaster. The experience gained by engineers over some 200 years of disasters and brushes with disaster is expressed in the extensive archival literature, national codes, and procedural documentation found in larger companies. However, the advantage of the richness in the behavior of shells is that the way is always open for innovation. In this survey, we present a broad overview of the dynamic response of shell structures. The intention is to provide an understanding of the basic themes behind the detailed codes and stimulate, not restrict, positive innovation. Such understanding is also crucial for the correct computation of shell structures by any computer code. The physics dictates that the thin shell structure offers a challenge for analysis and computation. Shell response can be generally categorized by states of extension, inextensional bending, edge bending, and edge transverse shear. Simple estimates for the magnitudes of stress, deformation, and resonance in the extensional and inextensional states are provided by ring response. Several shell examples demonstrate the different states and combinations. For excitation frequency above the extensional resonance, such as in impact and acoustic excitation, a fine mesh is needed over the entire shell surface. For this range, modal and implicit methods are of limited value. The example of a sphere impacting a rigid surface shows that plastic unloading occurs continuously. Thus, there are no short cuts; the complete material behavior must be included.

  4. Recent Developments in No-Core Shell-Model Calculations

    Energy Technology Data Exchange (ETDEWEB)

    Navratil, P; Quaglioni, S; Stetcu, I; Barrett, B R

    2009-03-20

    We present an overview of recent results and developments of the no-core shell model (NCSM), an ab initio approach to the nuclear many-body problem for light nuclei. In this aproach, we start from realistic two-nucleon or two- plus three-nucleon interactions. Many-body calculations are performed using a finite harmonic-oscillator (HO) basis. To facilitate convergence for realistic inter-nucleon interactions that generate strong short-range correlations, we derive effective interactions by unitary transformations that are tailored to the HO basis truncation. For soft realistic interactions this might not be necessary. If that is the case, the NCSM calculations are variational. In either case, the ab initio NCSM preserves translational invariance of the nuclear many-body problem. In this review, we, in particular, highlight results obtained with the chiral two- plus three-nucleon interactions. We discuss efforts to extend the applicability of the NCSM to heavier nuclei and larger model spaces using importance-truncation schemes and/or use of effective interactions with a core. We outline an extension of the ab initio NCSM to the description of nuclear reactions by the resonating group method technique. A future direction of the approach, the ab initio NCSM with continuum, which will provide a complete description of nuclei as open systems with coupling of bound and continuum states is given in the concluding part of the review.

  5. Shell effects in the superasymmetric fission

    CERN Document Server

    Mirea, M

    2002-01-01

    A new formalism based on the Landau-Zener promotion mechanism intends to explain the fine structure of alpha and cluster decay. The analysis of this phenomenon is accomplished by following the modality in which the shells are reorganized during the decay process beginning with the initial ground state of the parent towards the final configuration of two separated nuclei. A realistic level scheme is obtained in the framework of the superasymmetric two-center shell model. (author)

  6. Correlations between neutrons and protons near Fermi surface and $Q_{\\alpha}$ of super-heavy nuclei

    CERN Document Server

    Wang, Ning; Wu, Xizhen; Meng, Jie

    2015-01-01

    The shell corrections and shell gaps in nuclei are systematically studied with the latest Weizs\\"acker-Skyrme (WS4) mass model. We find that most of asymmetric nuclei with (sub)-shell closures locate along the shell stability line (SSL), $N=1.37Z+13.5$, which might be due to a strong correlation between neutrons and protons near Fermi surface. The double magicity of nuclei $^{46}$Si and $^{78}$Ni is predicted according to the corresponding shell gaps, shell corrections and nuclear deformations. The unmeasured super-heavy nuclei $^{296}$118 and $^{298}$120, with relatively large shell gaps and shell corrections, also locate along the SSL, whereas the traditional magic nucleus $^{298}$Fl evidently deviates from the line. The $\\alpha$-decay energies of super-heavy nuclei with $Z=113-126$ are simultaneously investigated by using the WS4 model together with the radial basis function corrections. For super-heavy nuclei with large shell corrections, the smallest $\\alpha$-decay energy for elements $Z=116$, 117 and 11...

  7. Mirror energy difference and the structure of loosely bound proton-rich nuclei around A = 20

    CERN Document Server

    Yuan, Cenxi; Xu, Furong; Suzuki, Toshio; Otsuka, Takaharu

    2014-01-01

    The properties of loosely bound proton-rich nuclei around A = 20 are investigated within the framework of nuclear shell model. In these nuclei, the strength of the effective interactions involving the loosely bound proton s1=2 orbit are significantly reduced in comparison with those in their mirror nuclei. We evaluate the reduction of the effective interaction by calculating the monopole-baseduniversal interaction (VMU) in the Woods-Saxon basis. The shell-model Hamiltonian in the sd shell, such as USD, can thus be modified to reproduce the binding energies and energy levels of the weakly bound proton-rich nuclei around A = 20. The effect of the reduction of the effective interaction on the structure and decay properties of these nuclei is also discussed.

  8. GDR in Hot Nuclei: New Measurements

    Science.gov (United States)

    Camera, F.; Kmiecik, M.; Wieland, O.; Benzoni, G.; Bracco, A.; Brambilla, S.; Crespi, F.; Mason, P.; Moroni, A.; Million, B.; Leoni, S.; Maj, A.; Styczen, J.; Brekiesz, M.; Meczynski, W.; Zieblinski, M.; Gramegna, F.; Barlini, S.; Kravchuk, V. L.; Lanchais, A. L.; Mastinu, P. F.; Bruno, M.; D'Agostino, M.; Geraci, E.; Ordine, A.; Casini, G.; Chiari, M.

    2005-04-01

    The measured properties of the Giant Dipole Resonance in hot rotating nuclei are successfully described with the model of thermal fluctuations, even though there are still some open problems especially at very low (T 2.5MeV) temperatures and missing data in some mass regions. Recent experimental works have addressed more specific problems regarding the nuclear shape and its behaviour in very particular and delimited phase space regions. In this paper will be discussed new exclusive measurements of the GDR γ decay in heavy 216Rn nuclei (where the shape of nuclei surviving fission have been probed) and some preliminary data on the 132Ce nuclei at very high excitation energy.

  9. Pro duction of Exotic Nuclei in Low-Energy Multi-Nucleon Transfer Reactions

    Institute of Scientific and Technical Information of China (English)

    VI Zagrebaev; Walter Greiner

    2015-01-01

    Multinucleon transfer processes in low-energy heavy ion collisions open a new field of re-search in nuclear physics, namely, production and studying properties of heavy neutron rich nuclei. This not-yet-explored area of the nuclear map is extremely important for understanding the astrophysical nu-cleosynthesis and the origin of heavy elements. Beams of very heavy U-like ions are needed to produce new long-living isotopes of transfermium and superheavy elements located very close to the island of sta-bility. The calculated cross sections are high enough to perform the experiments at available accelerators. Beams of medium-mass ions (such as 136Xe, 192Os, 198Pt) can be used for the production of neutron rich nuclei located along the neutron closed shell N=126 (the last waiting point) having the largest impact on the astrophysical r-process. The Low-energy multinucleon transfer reactions is a very efficient tool also for the production and spectroscopic study of light exotic nuclei. The corresponding cross sections are 2 or 3 orders of magnitude larger as compared with high energy fragmentation reactions.

  10. Discrimination between closed and open shell pistachio nuts using machine vision%基于机器视觉的开心果闭壳与开壳识别

    Institute of Scientific and Technical Information of China (English)

    郭晓伟

    2011-01-01

    To improve the quality of pistachio nuts, it is necessary to remove the closed shell pistachio nuts. A single row equally spacing method was taken to carry the pistachio nuts on the conveyor belt, and every pistachio nut image was captured by camera during the transmission. Then the image processing algorithm was used to detect whether its shell was open or not.Finally, gas nozzle, which was at the end of the conveyor belt, was used to blow away the closed shell pistachio nuts.Pistachio image was reduced to 0.2 times, and then the centroid of binary pistachio image was searched. After that, three horizontal pixel lines were described from the binary pistachio image, which was positioned in the centroid of pistachio, the middle of the upper part of pistachio and the middle of the lower part of pistachio. The gray value changes of all pixels of three lines were calculated respectively, and the features of those three pixel lines were integrated to judge whether the pistachio shell was open or not. Experiment results prove that the correct discrimination rates of the open shell pistachio nuts and the closed shell pistachio nuts are 93% and 100% respectively.%为从开心果中选出开壳果和去除闭壳果以提高开心果的品质.采用以单排等间距方式在传送带上输送开心果,输送过程中用摄像头拍摄每个开心果的图像,传输至电脑,经图像处理算法识别出开心果壳是否裂开,最后在传送带末端利用气嘴吹走闭壳果实以实现开心果自动分级.开心果图像缩小至原来的0.2倍,然后寻找出二值化图像中开心果的质心,再在开心果的质心、上半部分二分之一和下半部分二分之一处各取横向像素线,分别求取3条像素线上所有像素点灰度值变化之和,最后每个开心果综合3条像素线特征判断开心果是否开壳.实验证明开心果开壳果正确识别率为93%,闭壳果正确识别率达100%.

  11. From heavy nuclei to super-heavy nuclei; Des noyaux lourds aux super-lourds

    Energy Technology Data Exchange (ETDEWEB)

    Theisen, Ch

    2003-01-01

    The existence of super-heavy nuclei has been predicted nearly fifty years ago. Due to the strong coulomb repulsion, the stabilisation of these nuclei is possible only through shell effects. The reasons for this fragile stability, as well as the theoretical predictions concerning the position of the island of stability are presented in the first part of this lecture. In the second part, experiments and experimental techniques which have been used to synthesize or search for super-heavy elements are described. Spectroscopic studies performed in very heavy elements are presented in the following section. We close this lecture with techniques that are currently being developed in order to reach the superheavy island and to study the structure of very-heavy nuclei. (author)

  12. Difference in moments of inertia and paring interaction strength in superdeformed nuclei

    Institute of Scientific and Technical Information of China (English)

    雷奕安; 林纯镇; 曾谨言

    1997-01-01

    The difference in the bandhead moments of inertia between the superdeformed (SD) band 194Hg(1) and the two-quasiparticle SD bands 194Hg(2,3) was investigated using the particle-number-conserving treatment for the cranked shell model Hamiltonian, and the pairing interaction strength in SD nuclei is estimated to be much weaker than that in normally deformed nuclei.

  13. Relativistic Pseudospin Symmetry as a Supersymmetric Pattern in Nuclei

    CERN Document Server

    Leviatan, A

    2004-01-01

    Shell-model states involving several pseudospin doublets and ``intruder'' levels in nuclei, are combined into larger multiplets. The corresponding single-particle spectrum exhibits a supersymmetric pattern whose origin can be traced to the relativistic pseudospin symmetry of a nuclear mean-field Dirac Hamiltonian with scalar and vector potentials.

  14. Auxiliary-field quantum Monte Carlo methods in nuclei

    CERN Document Server

    Alhassid, Y

    2016-01-01

    Auxiliary-field quantum Monte Carlo methods enable the calculation of thermal and ground state properties of correlated quantum many-body systems in model spaces that are many orders of magnitude larger than those that can be treated by conventional diagonalization methods. We review recent developments and applications of these methods in nuclei using the framework of the configuration-interaction shell model.

  15. Shell supports

    DEFF Research Database (Denmark)

    Almegaard, Henrik

    2004-01-01

    A new statical and conceptual model for membrane shell structures - the stringer system - has been found. The principle was first published at the IASS conference in Copenhagen (OHL91), and later the theory has been further developed (ALMO3)(ALMO4). From the analysis of the stringer model it can...... be concluded that all membrane shells can be described by a limited number of basic configurations of which quite a few have free edges....

  16. Towards unified description of shell evolution — Takaharu Otsuka's achievements

    Science.gov (United States)

    Utsuno, Y.

    2013-07-01

    Recent studies on exotic nuclei have rapidly advanced the understanding of the evolution of shell structure, to which Takaharu Otsuka has made remarkable contributions particularly in terms of the nuclear force. This paper presents a brief survey of his achievements, focused on the concept of shell evolution due to the tensor force and the three-nucleon force and on related shell-model works.

  17. Non-empirical Prediction of the Photophysical and Magnetic Properties of Systems with Open d- and f-Shells Based on Combined Ligand Field and Density Functional Theory (LFDFT).

    Science.gov (United States)

    Daul, Claude

    2014-09-01

    Despite the important growth of ab initio and computational techniques, ligand field theory in molecular science or crystal field theory in condensed matter offers the most intuitive way to calculate multiplet energy levels arising from systems with open shells d and/or f electrons. Over the past decade we have developed a ligand field treatment of inorganic molecular modelling taking advantage of the dominant localization of the frontier orbitals within the metal-sphere. This feature, which is observed in any inorganic coordination compound, especially if treated by Density Functional Theory calculation, allows the determination of the electronic structure and properties with a surprising good accuracy. In ligand field theory, the theoretical concepts consider only a single atom center; and treat its interaction with the chemical environment essentially as a perturbation. Therefore success in the simple ligand field theory is no longer questionable, while the more accurate molecular orbital theory does in general over-estimate the metal-ligand covalence, thus yields wave functions that are too delocalized. Although LF theory has always been popular as a semi-empirical method when dealing with molecules of high symmetry e.g. cubic symmetry where the number of parameters needed is reasonably small (3 or 5), this is no more the case for molecules without symmetry and involving both an open d- and f-shell (# parameters ∼90). However, the combination of LF theory and Density Functional (DF) theory that we introduced twenty years ago can easily deal with complex molecules of any symmetry with two and more open shells. The accuracy of these predictions from 1(st) principles achieves quite a high accuracy (<5%) in terms of states energies. Hence, this approach is well suited to predict the magnetic and photo-physical properties arbitrary molecules and materials prior to their synthesis, which is the ultimate goal of each computational chemist. We will illustrate the

  18. Population of rotational bands in superheavy nuclei

    Directory of Open Access Journals (Sweden)

    Antonenko N.V.

    2012-02-01

    Full Text Available Using the statistical approach, we study the population of ground-state rotational bands of superheavy nuclei produced in the fusion-evaporation reactions 208Pb(48Ca, 2n254No, 206Pb(48Ca, 2n252No, and 204Hg(48Ca, 2n250Fm. We calculate relative intensities of E2-transitions between the rotational states and entry spin distributions of the residual nuclei, evaporation residue cross sections, and excitation functions for these reactions. Fermi-gas model is used for the calculation of level density, and damping of shell effects both with excitation energy and angular momentum is taking into account. The results are in a good agreement with the experiment data.

  19. Collective properties of drip-line nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Hamamoto, I. [Univ. of Lund (Sweden); Sagawa, H. [Univ. of Aizu, Fukushima (Japan)

    1996-12-31

    Performing the spherical Hartree-Fock (HF) calculations with Skyrme interactions and, then, using RPA solved in the coordinate space with the Green`s function method, the authors have studied the effect of the unique shell structure as well as the very low particle threshold on collective modes in drip line nuclei. In this method a proper strength function in the continuum is obtained, though the spreading width of collective modes is not included. They have examined also one-particle resonant states in the obtained HF potential. Unperturbed particle-hole (p-h) response functions are carefully studied, which contain all basic information on the exotic behaviour of the RPA strength function in drip line nuclei.

  20. Quarks in finite nuclei

    CERN Document Server

    Guichon, P A M; Thomas, A W

    1996-01-01

    We describe the development of a theoretical description of the structure of finite nuclei based on a relativistic quark model of the structure of the bound nucleons which interact through the (self-consistent) exchange of scalar and vector mesons.

  1. Probing Chiral Interactions in Light Nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Nogga, A; Barrett, B R; Meissner, U; Witala, H; Epelbaum, E; Kamada, H; Navratil, P; Glockle, W; Vary, J P

    2004-01-08

    Chiral two- and three-nucleon interactions are studied in a few-nucleon systems. We investigate the cut-off dependence and convergence with respect to the chiral expansion. It is pointed out that the spectra of light nuclei are sensitive to the three-nucleon force structure. As an example, we present calculations of the 1{sup +} and 3{sup +} states of {sup 6}Li using the no-core shell model approach. The results show contributions of the next-to-next-to-leading order terms to the spectra, which are not correlated to the three-nucleon binding energy prediction.

  2. The Structure of Nuclei Far from Stability

    Energy Technology Data Exchange (ETDEWEB)

    Zganjar, E.F.

    1999-02-25

    From among a number of important nuclear structure results that have emerged from our research program during the past few years, two stand out as being of extra significance. These are: (a) the identification of a diabatic coexisting structure in {sup 187}Au which arises solely from differences in proton occupation of adjacent oscillator shells, and (b) the realization of a method for estimating EO strength in nuclei and the resulting prediction that the de-excitation of superdeformed bands may proceed, in some cases, by strong EO transitions.

  3. Ground State Properties of Neutron Magic Nuclei

    CERN Document Server

    Saxena, G

    2016-01-01

    A systematic study of the ground state properties of the entire chains of even even neutron magic nuclei represented by isotones of traditional neutron magic numbers N = 8, 20, 40, 50, 82 and 126 has been carried out using relativistic mean field (rmf) plus Bardeen Cooper Schrieffer (BCS) approach. Our present investigation includes deformation, binding energy, two proton separation energy, single particle energy, rms radii along with proton and neutron density profiles, etc. Several of these results are compared with the results calculated using non relativistic approach (Skyrme Hartree Fock method) along with available experimental data and indeed they are found with excellent agreement. In addition, the possible locations of the proton and neutron drip lines, the (Z,N) values for the new shell closures, disappearance of traditional shell closures as suggested by the detailed analyzes of results are also discussed in detail.

  4. NEW EQUATIONS OF STATE BASED ON THE LIQUID DROP MODEL OF HEAVY NUCLEI AND QUANTUM APPROACH TO LIGHT NUCLEI FOR CORE-COLLAPSE SUPERNOVA SIMULATIONS

    Energy Technology Data Exchange (ETDEWEB)

    Furusawa, Shun; Yamada, Shoichi [Advanced Research Institute for Science and Engineering, Waseda University, 3-4-1 Okubo, Shinjuku, Tokyo 169-8555 (Japan); Sumiyoshi, Kohsuke [Numazu College of Technology, Ooka 3600, Numazu, Shizuoka 410-8501 (Japan); Suzuki, Hideyuki, E-mail: furusawa@heap.phys.waseda.ac.jp [Faculty of Science and Technology, Tokyo University of Science, Yamazaki 2641, Noda, Chiba 278-8510 (Japan)

    2013-08-01

    We construct new equations of state for baryons at subnuclear densities for the use in core-collapse simulations of massive stars. The abundance of various nuclei is obtained together with thermodynamic quantities. A model free energy is constructed, based on the relativistic mean field theory for nucleons and the mass formula for nuclei with the proton number up to {approx}1000. The formulation is an extension of the previous model, in which we adopted the liquid drop model to all nuclei under the nuclear statistical equilibrium. We reformulate the new liquid drop model so that the temperature dependences of bulk energies could be taken into account. Furthermore, we extend the region in the nuclear chart, in which shell effects are included, by using theoretical mass data in addition to experimental ones. We also adopt a quantum-theoretical mass evaluation of light nuclei, which incorporates the Pauli- and self-energy shifts that are not included in the ordinary liquid drop model. The pasta phases for heavy nuclei are taken into account in the same way as in the previous model. We find that the abundances of heavy nuclei are modified by the shell effects of nuclei and temperature dependence of bulk energies. These changes may have an important effect on the rates of electron captures and coherent neutrino scatterings on nuclei in supernova cores. The abundances of light nuclei are also modified by the new mass evaluation, which may affect the heating and cooling rates of supernova cores and shocked envelopes.

  5. Interweaving of elementary modes of excitation in superfluid nuclei through particle-vibration coupling: Quantitative account of the variety of nuclear structure observables

    Science.gov (United States)

    Idini, A.; Potel, G.; Barranco, F.; Vigezzi, E.; Broglia, R. A.

    2015-09-01

    A complete characterization of the structure of nuclei can be obtained by combining information arising from inelastic scattering, Coulomb excitation, and γ -decay, together with one- and two-particle transfer reactions. In this way it is possible to probe both the single-particle and collective components of the nuclear many-body wave function resulting from the coupling of these modes and, as a result, diagonalizing the low-energy Hamiltonian. We address the question of how accurately such a description can account for experimental observations in the case of superfluid nuclei. Our treatment goes beyond the traditional approach, in which these properties are calculated separately, and most often for systems near closed shells, based on perturbative approximations (weak coupling). It is concluded that renormalizing empirically and on equal footing bare single-particle and collective motion of open-shell nuclei in terms of self-energy (mass) and vertex corrections (screening), as well as particle-hole and pairing interactions through particle-vibration coupling (PVC), leads to a detailed, quantitative account of the data, constraining the possible values of the k mass, of the 1S0 bare N N interaction, and of the PVC strengths within a rather narrow window.

  6. Survey of excited state neutron spectroscopic factors for Z=8-28 nuclei

    CERN Document Server

    Tsang, M B; Su, S C; Dai, J Y; Horoi, M; Liu, H; Lynch, W G; Warren, S

    2008-01-01

    We have extracted 565 neutron spectroscopic factors of the sd and fp shell nuclei by systematically analyzing more than 2000 measured (d,p) angular distributions. We are able to compare 125 of the extracted spectroscopic factors to values predicted by large-basis shell-model calculations and evaluate the accuracies of spectroscopic factors predicted by different shell-model interactions in these regions. We find that the spectroscopic factors predicted for most excited states of sd-shell nuclei using the latest USDB or USDA interactions agree with the experimental values. For fp shell nuclei, the inability of the current models to account for the core excitation and fragmentation of the states leads to considerable discrepancies. The agreement between data and shell-model predictions for Ni isotopes is not better than a factor of two using either the GXPF1A or the XT interaction. The systematics of spectroscopic factors for the sd-shell nuclei and Ni isotopes indicate that small spectroscopic values predicted...

  7. Are the nuclei beyond 132Sn very exotic?

    Science.gov (United States)

    Lozeva, R.; Naïdja, H.; Nowacki, F.; Odahara, A.; Moon, C.-B.; NP1112-RIBF87 Collaboration

    2016-06-01

    The term exotic nucleus is used for nuclei that have different from normal behavior. However, it turns out that the term normal is valid only for nuclei close to stability and more particularly for regions close to double-shell closures. As long as one drives away in the neutron-rich nuclei, especially at intermediate mass number, interplay between normal single-particle and many collective particle-hole excitations compete. In some cases with the addition of neutrons, these may turn to evolve as a skin, acting against the core nucleus that may also influence its shell evolution. Knowledge of these nuclear ingredients is especially interesting beyond the doubly-magic 132Sn, however a little is known on how the excitations modes develop with the addition of both protons and neutrons. Especially for the Sb nuclei, where one gradually increases these valence particles, the orbital evolution and its impact on exoticness is very intriguing. Experimental studies were conducted on several such isotopes using isomer and, β-decay spectroscopy at RIBF within EURICA. In particular, new data on 140Sb and 136Sb are examined and investigated in the framework of shell model calculations.

  8. Stress Concentration Analysis of Reinforced Cylindrical Shells with Large Opening%圆柱壳大开孔补强的应力集中分析

    Institute of Scientific and Technical Information of China (English)

    舒斌; 胡刚义; 肖伟; 张元盛

    2011-01-01

    Combined with practical engineering, stress concentration on the reinforcement of pressure hull of submarine with large opening was studied.Different forms of reinforcement were investigated by the Finite Element Method (FEM) and rules of thumb.Models were constructed and the stress concentration factors were worked out.By comparing and analyzing the results from these two methods, it shows that the bending hoop stress of opening where lies in maximum hoop membrane stress cannot be ignored when the opening stiffened by coaming.The calculations also prove effective in reinforcement of structural design of large openings.%针对潜艇耐压壳体上大开孔补强处的应力集中现象,结合工程实际问题,采用规范和有限元法对潜艇耐压壳体上大开孔不同补强形式进行了研究,建立了相应的模型,并求出了应力集中系数.通过对两种方法的计算结果进行分析比较,发现当围壁加强时,最大周向应力处的弯曲应力不容忽视.结果说明,用有限单元法进行大开孔补强结构设计是合理、有效的,是对规范计算的完善和补充.

  9. Molecular outflows in starburst nuclei

    CERN Document Server

    Roy, Arpita; Sharma, Prateek; Shchekinov, Yuri

    2016-01-01

    Recent observations have detected molecular outflows in a few nearby starburst nuclei. We discuss the physical processes at work in such an environment in order to outline a scenario that can explain the observed parameters of the phenomenon, such as the molecular mass, speed and size of the outflows. We show that outflows triggered by OB associations, with $N_{OB}\\ge 10^5$ (corresponding to a star formation rate (SFR)$\\ge 1$ M$_{\\odot}$ yr$^{-1}$ in the nuclear region), in a stratified disk with mid-plane density $n_0\\sim 200\\hbox{--}1000$ cm$^{-3}$ and scale height $z_0\\ge 200 (n_0/10^2 \\, {\\rm cm}^{-3})^{-3/5}$ pc, can form molecules in a cool dense and expanding shell. The associated molecular mass is $\\ge 10^7$ M$_\\odot$ at a distance of a few hundred pc, with a speed of several tens of km s$^{-1}$. We show that a SFR surface density of $10 \\le \\Sigma_{SFR} \\le 50$ M$_\\odot$ yr$^{-1}$ kpc$^{-2}$ favours the production of molecular outflows, consistent with observed values.

  10. Reactions with fast radioactive beams of neutron-rich nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Aumann, T. [Gesellschaft fuer Schwerionenforschung mbH, Darmstadt (Germany)

    2005-11-01

    The neutron dripline has presently been reached only for the lightest nuclei up to the element oxygen. In this region of light neutron-rich nuclei, scattering experiments are feasible even for dripline nuclei by utilizing high-energy secondary beams produced by fragmentation. In the present article, reactions of high-energy radioactive beams will be exemplified using recent experimental results mainly derived from measurements of breakup reactions performed at the LAND and FRS facilities at GSI and at the S800 spectrometer at the NSCL. Nuclear and electromagnetically induced reactions allow probing different aspects of nuclear structure at the limits of stability related to the neutron-proton asymmetry and the weak binding close to the dripline. Properties of the valence-neutron wave functions are studied in the one-neutron knockout reaction, revealing the changes of shell structure when going from the beta-stability line to more asymmetric loosely bound neutron-rich systems. The vanishing of the N=8 shell gap for neutron-rich systems like {sup 11}Li and {sup 12}Be, or the new closed N=14, 16 shells for the oxygen isotopes are examples. The continuum of weakly bound nuclei and halo states can be studied by inelastic scattering. The dipole response, for instance, is found to change dramatically when going away from the valley of stability. A redistribution of the dipole strength towards lower excitation energies is observed for neutron-rich nuclei, which partly might be due to a new collective excitation mode related to the neutron-proton asymmetry. Halo nuclei in particular show strong dipole transitions to the continuum at the threshold, being directly related to the ground-state properties of the projectile. Finally, an outlook on future experimental prospects is given. (orig.)

  11. Anharmonic vibrations in nuclei

    CERN Document Server

    Fallot, M; Andrés, M V; Catara, F; Lanza, E G; Scarpaci, J A; Chomaz, Ph.

    2003-01-01

    In this letter, we show that the non-linearitites of large amplitude motions in atomic nuclei induce giant quadrupole and monopole vibrations. As a consequence, the main source of anharmonicity is the coupling with configurations including one of these two giant resonances on top of any state. Two-phonon energies are often lowered by one or two MeV because of the large matrix elements with such three phonon configurations. These effects are studied in two nuclei, 40Ca and 208Pb.

  12. The shapes of nuclei

    CERN Document Server

    Bertsch, G F

    2016-01-01

    Gerry Brown initiated some early studies on the coexistence of different nuclear shapes. The subject has continued to be of interest and is crucial for understanding nuclear fission. We now have a very good picture of the potential energy surface with respect to shape degrees of freedom in heavy nuclei, but the dynamics remain problematic. In contrast, the early studies on light nuclei were quite successful in describing the mixing between shapes. Perhaps a new approach in the spirit of the old calculations could better elucidate the character of the fission dynamics and explain phenomena that current theory does not model well.

  13. Shell Evolutions and Nuclear Forces

    CERN Document Server

    Sorlin, O

    2014-01-01

    During the last 30 years, and more specifically during the last 10 years, many experiments have been carried out worldwide using different techniques to study the shell evolution of nuclei far from stability. What seemed not conceivable some decades ago became rather common: all known magic numbers that are present in the valley of stability disappear far from stability and are replaced by new ones at the drip line. By gathering selected experimental results, beautifully consistent pictures emerge, that very likely take root in the properties of the nuclear forces.The present manuscript describes some of these discoveries and proposes an intuitive understanding of these shell evolutions derived from observations. Extrapolations to yet unstudied regions, as where the explosive r-process nucleosynthesis occurs, are proposed. Some remaining challenges and puzzling questions are also addressed.

  14. 7 CFR 51.2542 - U.S. Artificially Opened.

    Science.gov (United States)

    2010-01-01

    ... STANDARDS) United States Standards for Grades of Pistachio Nuts in the Shell § 51.2542 U.S. Artificially Opened. “U.S. Artificially Opened” consists of artificially opened pistachio nuts in the shell which...

  15. Electric dipole moments of neutron-odd nuclei

    Science.gov (United States)

    Fujita, Takehisa; Oshima, Sachiko

    2012-09-01

    We systematically calculate the electric dipole moments (EDMs) of neutron-odd nuclei with even protons in a phenomenological shell model picture. We first derive the relation between the EDM and the magnetic moment operators by making use of the core polarization scheme. This relation enables us to calculate the EDM of neutron-odd nuclei using the experimental values of the magnetic moments. From the calculations, one may find the best atomic system suitable for future EDM experiments where the estimations are made for doubly ionized atoms.

  16. Pressure Shell Approach to Integrated Environmental Protection

    Science.gov (United States)

    Kennedy, Kriss J.

    2011-01-01

    The next generation of exploration mission human systems will require environmental protection such as radiation protection that is effective and efficient. In order to continue human exploration, habitat systems will require special shells to protect astronauts from hostile environments. The Pressure Shell Approach to integrated environmental (radiation) protection is a multi-layer shell that can be used for multifunctional environmental protection. Self-healing, self-repairing nano technologies and sensors are incorporated into the shell. This shell consists of multiple layers that can be tailored for specific environmental protection needs. Mainly, this innovation focuses on protecting crew from exposure to micrometeorites, thermal, solar flares, and galactic cosmic ray (GCR) radiation. The Pressure Shell Approach consists of a micrometeoroid and secondary ejecta protection layer; a thin, composite shell placed in between two layers that is non-structural; an open cavity layer that can be filled with water, regolith, or polyethylene foam; a thicker composite shell that is a structural load bearing that is placed between two layers; and a bladder coating on the interior composite shell. This multi-layer shell creates an effective radiation protection system. Most of its layers can be designed with the materials necessary for specific environments. In situ materials such as water or regolith can be added to the shell design for supplemental radiation protection.

  17. Spin Density Distribution in Open-Shell Transition Metal Systems: A Comparative Post-Hartree-Fock, Density Functional Theory, and Quantum Monte Carlo Study of the CuCl2 Molecule.

    Science.gov (United States)

    Caffarel, Michel; Giner, Emmanuel; Scemama, Anthony; Ramírez-Solís, Alejandro

    2014-12-09

    We present a comparative study of the spatial distribution of the spin density of the ground state of CuCl2 using Density Functional Theory (DFT), quantum Monte Carlo (QMC), and post-Hartree-Fock wave function theory (WFT). A number of studies have shown that an accurate description of the electronic structure of the lowest-lying states of this molecule is particularly challenging due to the interplay between the strong dynamical correlation effects in the 3d shell and the delocalization of the 3d hole over the chlorine atoms. More generally, this problem is representative of the difficulties encountered when studying open-shell metal-containing molecular systems. Here, it is shown that qualitatively different results for the spin density distribution are obtained from the various quantum-mechanical approaches. At the DFT level, the spin density distribution is found to be very dependent on the functional employed. At the QMC level, Fixed-Node Diffusion Monte Carlo (FN-DMC) results are strongly dependent on the nodal structure of the trial wave function. Regarding wave function methods, most approaches not including a very high amount of dynamic correlation effects lead to a much too high localization of the spin density on the copper atom, in sharp contrast with DFT. To shed some light on these conflicting results Full CI-type (FCI) calculations using the 6-31G basis set and based on a selection process of the most important determinants, the so-called CIPSI approach (Configuration Interaction with Perturbative Selection done Iteratively) are performed. Quite remarkably, it is found that for this 63-electron molecule and a full CI space including about 10(18) determinants, the FCI limit can almost be reached. Putting all results together, a natural and coherent picture for the spin distribution is proposed.

  18. Bio-relevant dissolution testing of hard capsules prepared from different shell materials using the dynamic open flow through test apparatus.

    Science.gov (United States)

    Garbacz, Grzegorz; Cadé, Dominique; Benameur, Hassan; Weitschies, Werner

    2014-06-16

    Current compendial dissolution and disintegrating testing is unable to mimic physiological conditions affecting gastric drug release from immediate release dosage forms. In order to obtain more realistic data, a novel test setup was developed that we term a 'dynamic open flow through test apparatus'. It is based on the previously described dissolution stress test device and attempts to simulate the intra-gastric dissolution conditions pertinent to immediate release dosage forms administered under fasting conditions with respect to flow rates, intra-gastric temperature profiles and gastric motility. The concept of the dynamic open flow through test apparatus has been tested using five different types of hard capsules: conventional hard gelatin capsules (HGC), three hypromellose based capsules (Vcaps, Vcaps Plus and DRcaps) and pullulan based capsules (Plantcaps). These were of different sizes but all contained 100mg caffeine in each formulation, adjusted to avoid buoyancy by addition of excipient. When the capsules were stressed in the apparatus under the dynamic flow conditions applying mild pressure simulating gastric motility, release from release from Vcaps Plus, Vcaps and Plantcaps capsules was very well comparable to HGC. Capsules are usually swallowed with cold water and the temperature dependency of release from gelatin was noted as a significant factor, since heat exchange in the stomach is slow. Copyright © 2013 Elsevier B.V. All rights reserved.

  19. Shell model spectroscopy far from stability

    Science.gov (United States)

    Poves, A.

    2017-08-01

    I will discuss the impact of the research on exotic nuclei carried out at ISOLDE and later on, following its impulse, in many laboratories worldwide, in our present knowledge of the nuclear dynamics. I will put particular emphasis on the occurrence of islands of inversion (IoI) at several magic numbers for the neutrons, far from stability. I will also discuss the appearance of new local shell closures in the calcium and silicon isotopic chains, and qualify their status as new doubly magic nuclei. This article belongs to the Focus on Exotic Beams at ISOLDE: A Laboratory Portrait special issue.

  20. Elusive active galactic nuclei

    NARCIS (Netherlands)

    Maiolino, R; Comastri, A; Gilli, R; Nagar, NM; Bianchi, S; Boker, T; Colbert, E; Krabbe, A; Marconi, A; Matt, G; Salvati, M

    2003-01-01

    A fraction of active galactic nuclei do not show the classical Seyfert-type signatures in their optical spectra, i.e. they are optically 'elusive'. X-ray observations are an optimal tool to identify this class of objects. We combine new Chandra observations with archival X-ray data in order to obtai

  1. Influence of Neutron Shell Closure (Nc=126) on Prescission Particle Emission of Fissioning Systems 216,224Th

    Institute of Scientific and Technical Information of China (English)

    叶巍

    2003-01-01

    The effect of neutron shell closure Nc = 126 on the prescission-particle emission of 216Th and 224Th nuclei is investigated within the framework of an extensive Smoluchowski equation. It is found that there is a large difference in the prescission neutron multiplicity for the two Th nuclei, indicating a strong shell effect in neutron emission. Moreover, shell effects on particle emission are also investigated as functions of excitation energy,angular momentum and nuclear viscosity. The results show that with increasing excitation energy shell effects in prefission neutron evolve from continual strength to gradual weakness. Both high angular momenta and low viscosity weaken the shell effects on the particle emission.

  2. Decay of Hot Nuclei at Low Spins Produced by Antiproton-Annihilation in Heavy Nuclei

    CERN Multimedia

    2002-01-01

    % PS208 \\\\ \\\\ The objective of the experiment is to study (i) the thermal excitation energy distribution of antiproton-induced reactions in heavy nuclei and (ii) the decay properties of hot nuclei at low spins via evaporation, multifragmentation and fission as a function of excitation energy. The experimental set-up consists of 4-$\\pi$ detectors: the Berlin Neutron Ball~(BNB) which is a spherical shell of gadolinium-loaded scintillator liquid with an inner and outer diameter of 40 and 160~cm, respectively. This detector counts the number of evaporated neutrons in each reaction. Inside BNB there is a 4-$\\pi$ silicon ball~(BSIB) with a diameter of 20~cm consisting of 162 detectors which measure energy and multiplicity of all emitted charged nuclear particles. The particles are identified via time of flight, energy and pulse shape correlations.

  3. Shape Deformations in Atomic Nuclei

    CERN Document Server

    Hamamoto, Ikuko

    2011-01-01

    The ground states of some nuclei are described by densities and mean fields that are spherical, while others are deformed. The existence of non-spherical shape in nuclei represents a spontaneous symmetry breaking.

  4. Ultra High Energy Nuclei Propagation

    CERN Document Server

    Aloisio, Roberto

    2008-01-01

    We discuss the problem of ultra high energy nuclei propagation in astrophysical backgrounds. We present a new analytical computation scheme based on the hypothesis of continuos energy losses in a kinetic formulation of the particles propagation. This scheme enables the computation of the fluxes of ultra high energy nuclei as well as the fluxes of secondaries (nuclei and nucleons) produced by the process of photo-disintegration suffered by nuclei.

  5. Level density and shape changes in excited sd shell nuclei

    Indian Academy of Sciences (India)

    S Santosh Kumar

    2008-07-01

    In the present calculation we have used the Monte Carlo method of generating collective spin and total energy of the nucleus for various configurations of the system with 0 single particle states available for n number of particles. The different configurations (arrangements of occupied single particle states) leading to a particular energy and spin are then collected to get the density of states for the given energy and spin . We find that if we use the cranked Nilsson model single particle states for the rotational frequency = 0.0ħω, 0.05ħω and 0.1ħω there is a shift in the maximum density of states max with a tendency for the system to become more oblate or prolate depending on the shift in the maximum density of states as the angular momentum decreases or increases. The change in nuclear level density with collectivity, i.e. with the use of cranked Nilsson model single particle levels has been noticed.

  6. Multinucleon transfer reactions in closed-shell nuclei

    CERN Document Server

    Szilner, S; Corradi, L; Marginean, N; Pollarolo, G; Stefanini, A M; Beghini, S; Behera, B R; Fioretto, E; Gadea, A; Guiot, B; Latina, A; Mason, P; Montagnoli, G; Scarlassara, F; Trotta, M; de Angelis, G; Della Vedova, F; Farnea, E; Haas, F; Lenzi, S; Lunardi, S; Marginean, R; Menegazzo, R; Napoli, D R; Nespolo, M; Pokrovsky, I V; Recchia, F; Romoli, M; Salsac, M -D; Soic, N; Valiente-Dobon, J J

    2007-01-01

    Multinucleon transfer reactions in 40Ca+96Zr and 90Zr+208Pb have been measured at energies close to the Coulomb barrier in a high resolution gamma-particle coincidence experiment. The large solid angle magnetic spectrometer PRISMA coupled to the CLARA gamma-array has been employed. Trajectory reconstruction has been applied for the complete identification of transfer products. Mass and charge yields, total kinetic energy losses, gamma transitions of the binary reaction partners, and comparison of data with semiclassical calculations are reported. Specific transitions in 95Zr populated in one particle transfer channels are discussed in terms of particle-phonon couplings. The gamma decays from states in 42Ca in the excitation energy region expected from pairing vibrations are also observed.

  7. Fusion probability in heavy nuclei

    Science.gov (United States)

    Banerjee, Tathagata; Nath, S.; Pal, Santanu

    2015-03-01

    Background: Fusion between two massive nuclei is a very complex process and is characterized by three stages: (a) capture inside the potential barrier, (b) formation of an equilibrated compound nucleus (CN), and (c) statistical decay of the CN leading to a cold evaporation residue (ER) or fission. The second stage is the least understood of the three and is the most crucial in predicting yield of superheavy elements (SHE) formed in complete fusion reactions. Purpose: A systematic study of average fusion probability, PCN> , is undertaken to obtain a better understanding of its dependence on various reaction parameters. The study may also help to clearly demarcate onset of non-CN fission (NCNF), which causes fusion probability, PCN, to deviate from unity. Method: ER excitation functions for 52 reactions leading to CN in the mass region 170-220, which are available in the literature, have been compared with statistical model (SM) calculations. Capture cross sections have been obtained from a coupled-channels code. In the SM, shell corrections in both the level density and the fission barrier have been included. PCN> for these reactions has been extracted by comparing experimental and theoretical ER excitation functions in the energy range ˜5 %-35% above the potential barrier, where known effects of nuclear structure are insignificant. Results: PCN> has been shown to vary with entrance channel mass asymmetry, η (or charge product, ZpZt ), as well as with fissility of the CN, χCN. No parameter has been found to be adequate as a single scaling variable to determine PCN> . Approximate boundaries have been obtained from where PCN> starts deviating from unity. Conclusions: This study quite clearly reveals the limits of applicability of the SM in interpreting experimental observables from fusion reactions involving two massive nuclei. Deviation of PCN> from unity marks the beginning of the domain of dynamical models of fusion. Availability of precise ER cross sections

  8. Inner shell radial pin geometry and mounting arrangement

    Science.gov (United States)

    Leach, David; Bergendahl, Peter Allen

    2002-01-01

    Circumferentially spaced arrays of support pins are disposed through access openings in an outer turbine shell and have projections received in recesses in forward and aft sections of an inner turbine shell supported from the outer shell. The projections have arcuate sides in a circumferential direction affording line contacts with the side walls of the recesses and are spaced from end faces of the recesses, enabling radial and axial expansion and contraction of the inner shell relative to the outer shell. All loads are taken up in a tangential direction by the outer shell with the support pins taking no radial loadings.

  9. Injection mould for open-faced cellphone bottom shell%直板手机底壳注射模设计

    Institute of Scientific and Technical Information of China (English)

    梁国栋

    2012-01-01

    The forming process and key points in designing the structure of an injection mould for an open-faced cellphone were presented. The three-plate mould has three pin gates. The upended part at two sides was formed by slider in the fixed half and the one at the other two sides was formed in the moving half. Limit switch was applied to prevent the ejector rod and slider in the moving half from interference.%介绍了一款直板手机底壳的成型工艺与注射模结构设计要点,模具采用三板模结构,三点进浇,两面采用定模滑块成型倒扣,另外两面采用动模滑块成型倒扣,使用行程开关防止推杆与动模滑块干涉,实践证明模具结构合理,脱模顺利,塑件质量满足要求.

  10. Relativistic Brueckner-Hartree-Fock theory for finite nuclei

    CERN Document Server

    Shen, Shihang; Liang, Haozhao; Meng, Jie; Ring, Peter; Zhang, Shuangquan

    2016-01-01

    Starting with a bare nucleon-nucleon interaction, for the first time the full relativistic Brueckner-Hartree-Fock equations are solved for finite nuclei in a Dirac-Woods-Saxon basis. No free parameters are introduced to calculate the ground-state properties of finite nuclei. The nucleus $^{16}$O is investigated as an example. The resulting ground-state properties, such as binding energy and charge radius, are considerably improved as compared with the non-relativistic Brueckner-Hartree-Fock results and much closer to the experimental data. This opens the door for \\emph{ab initio} covariant investigations of heavy nuclei.

  11. Bubble nuclei; Noyaux Bulles

    Energy Technology Data Exchange (ETDEWEB)

    Legoll, F. [Service de Physique Theorique, CEA Centre d`Etudes de Saclay, 91 - Gif-sur-Yvette (France)

    1998-07-22

    For nuclei with very high electrical charge, the Coulomb field is expected to drive the protons away from the centre to the surface of the nucleus. Such a nucleus would be no more compact but look like a bubble. The goal of this work is to confirm this idea. We are interested in only the ground state of spherical nuclei. We use the Skyrme potential with the Sly4 parametrization to calculate the mean-field Hamiltonian. Paring correlations are described by a surface-active delta paring interaction. In its ground state the nucleus {sup A=900} X{sub Z=274} is shown to be a bubble. Another stable state is found with a little higher energy: it is also a bubble. (author) 11 refs., 18 figs., 33 tabs.

  12. Bubble nuclei; Noyaux Bulles

    Energy Technology Data Exchange (ETDEWEB)

    Legoll, F. [Service de Physique Theorique, CEA Centre d`Etudes de Saclay, 91 - Gif-sur-Yvette (France)

    1998-07-22

    For nuclei with very high electrical charge, the Coulomb field is expected to drive the protons away from the centre to the surface of the nucleus. Such a nucleus would be no more compact but look like a bubble. The goal of this work is to confirm this idea. We are interested in only the ground state of spherical nuclei. We use the Skyrme potential with the Sly4 parametrization to calculate the mean-field Hamiltonian. Paring correlations are described by a surface-active delta paring interaction. In its ground state the nucleus {sup A=900} X{sub Z=274} is shown to be a bubble. Another stable state is found with a little higher energy: it is also a bubble. (author) 11 refs., 18 figs., 33 tabs.

  13. Pro OpenSSH

    CERN Document Server

    Stahnke, Michael

    2006-01-01

    SSH, acronym for Secure Socket Shell, is for users and administrators wishing to establish secure communication between disparate networks. 'Pro OpenSSH', authored by two Fortune 100 system administrators, provides readers with a highly practical reference for configuring and deploying OpenSSH in their own environment.

  14. The study of the action of self-friction field on the atom and molecular structures by using combined Hartree-Fock-Roothaan theory for closed and open shells of any symmetry

    Science.gov (United States)

    Mamedov, B. A.; Çopuroğlu, E.

    2016-06-01

    In this work, we study the effects of self-friction field on the states of a single configuration of closed and open shells by using the Combined Hartree-Fock-Roothaan equations for atomic-molecular and nuclear systems. Here, we present a program that implements the evaluation of the various properties of atoms and molecular systems with respect to the various values of self-friction quantum numbers. An especially fast and accurate algorithm for the calculation of the self-friction multicenter molecular integrals is obtained by using one-range addition theorems. To demonstrate the action of self-friction field on the atomic and molecular systems we have performed the calculations of H2O, CH3, CH2 and NH3 molecules. For the derivations of the orbital, kinetic and total energies and linear combination coefficients, the results are given for various values of self-friction quantum numbers. For various values of self-friction quantum numbers the obtained results of the orbital, kinetic and total energies and linear combination coefficients have been analyzed.

  15. An assessment of pure, hybrid, meta, and hybrid-meta GGA density functional theory methods for open-shell systems: the case of the nonheme iron enzyme 8R-LOX.

    Science.gov (United States)

    Bushnell, Eric A C; Gauld, James W

    2013-01-15

    The performance of a range density functional theory functionals combined in a quantum mechanical (QM)/molecular mechanical (MM) approach was investigated in their ability to reliably provide geometries, electronic distributions, and relative energies of a multicentered open-shell mechanistic intermediate in the mechanism 8R-Lipoxygenase. With the use of large QM/MM active site chemical models, the smallest average differences in geometries between the catalytically relevant quartet and sextet complexes were obtained with the B3LYP(*) functional. Moreover, in the case of the relative energies between (4) II and (6) II, the use of the B3LYP(*) functional provided a difference of 0.0 kcal mol(-1). However, B3LYP(±) and B3LYP also predicted differences in energies of less than 1 kcal mol(-1). In the case of describing the electronic distribution (i.e., spin density), the B3LYP(*), B3LYP, or M06-L functionals appeared to be the most suitable. Overall, the results obtained suggest that for systems with multiple centers having unpaired electrons, the B3LYP(*) appears most well rounded to provide reliable geometries, electronic structures, and relative energies. Copyright © 2012 Wiley Periodicals, Inc.

  16. On Quasibound N* Nuclei

    CERN Document Server

    Kelkar, N G; Moskal, P

    2015-01-01

    The possibility for the existence of unstable bound states of the S11 nucleon resonance N$^*$(1535) and nuclei is investigated. These quasibound states are speculated to be closely related to the existence of the quasibound states of the eta mesons and nuclei. Within a simple model for the N N$^*$ interaction involving a pion and eta meson exchange, N$^*$-nucleus potentials for N*-$^3$He and N*-$^{24}$Mg are evaluated and found to be of a Woods-Saxon like form which supports two to three bound states. In case of N*-$^3$He, one state bound by only a few keV and another by 4 MeV is found. The results are however quite sensitive to the N N$^*$ $\\pi$ and N N$^*$ $\\eta$ vertex parameters. A rough estimate of the width of these states, based on the mean free path of the exchanged mesons in the nuclei leads to very broad states with $\\Gamma \\sim$ 80 and 110 MeV for N*-$^3$He and N*-$^{24}$Mg respectively.

  17. High spin spectroscopy of near spherical nuclei: Role of intruder orbitals

    Energy Technology Data Exchange (ETDEWEB)

    Bhattacharyya, S.; Bhattacharjee, T.; Mukherjee, G. [Variable Energy Cyclotron Centre, 1/AF Bidhan Nagar, Kolkata - 700064 (India); Chanda, S. [Fakir Chand College, Diamond Herbour, West Bengal (India); Banerjee, D.; Das, S. K.; Guin, R. [Radiochemistry Division, Variable Energy Cyclotron Centre, BARC, Kolkata - 700064 (India); Gupta, S. Das [Variable Energy Cyclotron Centre, 1/AF Bidhan Nagar, Kolkata - 700064, India and Saha Institute of Nuclear Physics, Kolkata-700064 (India); Pai, H. [Variable Energy Cyclotron Centre, 1/AF Bidhan Nagar, Kolkata - 700064, India and Institut für Kernphysik, Technische Universität Darmstadt, Schlossgartenstrasse 9, 64289 Darmstadt (Germany)

    2014-08-14

    High spin states of nuclei in the vicinity of neutron shell closure N = 82 and proton shell closure Z = 82 have been studied using the Clovere Ge detectors of Indian National Gamma Array. The shape driving effects of proton and neutron unique parity intruder orbitals for the structure of nuclei around the above shell closures have been investigated using light and heavy ion beams. Lifetime measurements of excited states in {sup 139}Pr have been done using pulsed-beam-γ coincidence technique. The prompt spectroscopy of {sup 207}Rn has been extended beyond the 181μs 13/2{sup +} isomer. Neutron-rich nuclei around {sup 132}Sn have been produced from proton induced fission of {sup 235}U and lifetime measurement of low-lying states of odd-odd {sup 132}I have been performed from offline decay.

  18. NIF Double Shell outer-shell experiments

    Science.gov (United States)

    Merritt, E. C.; Montgomery, D. S.; Kline, J. L.; Daughton, W. S.; Wilson, D. C.; Dodd, E. S.; Renner, D. B.; Cardenas, T.; Batha, S. H.

    2016-10-01

    At the core of the Double Shell concept is the kinetic energy transfer from the outer shell to the inner shell via collision. This collision sets both the implosion shape of the inner shell, from imprinting of the shape of the outer shell, as well as the maximum energy available to compress the DT fuel. Therefore, it is crucial to be able to control the time-dependent shape of the outer shell, such that the outer shell is nominally round at the collision time. We present the experiment results from our sub-scale ( 1 MJ) NIF outer-shell only shape tuning campaign, where we vary shape by changing a turn-on time delay between the same pulse shape on the inner and outer cone beams. This type of shape tuning is unique to this platform and only possible since the Double Shell design uses a single-shock drive (4.5 ns reverse ramp pulse). The outer-shell only targets used a 5.75 mm diameter standard near-vacuum NIF hohlraum with 0.032 mg/cc He gas fill, and a Be capsule with 0.4% uniform Cu dopant, with 242 um thick ablator. We also present results from a third outer-shell only shot used to measure shell trajectory, which is critical in determining the shell impact time. This work conducted under the auspices of the U.S. DOE by LANL under contract DE-AC52-06NA25396.

  19. Giant Monopole Resonance in even-A Cd isotopes, the asymmetry term in nuclear incompressibility, and the "softness" of Sn and Cd nuclei

    CERN Document Server

    Patel, D; Fujiwara, M; Akimune, H; Berg, G P A; Harakeh, M N; Itoh, M; Kawabata, T; Kawase, K; Nayak, B K; Ohta, T; Ouchi, H; Piekarewicz, J; Uchida, M; Yoshida, H P; Yosoi, M

    2012-01-01

    The isoscalar giant monopole resonance (ISGMR) in even-A Cd isotopes has been studied by inelastic ${\\alpha}$-scattering at 100 MeV/u and at extremely forward angles, including 0deg. The asymmetry term in the nuclear incompressibility extracted from the ISGMR in Cd isotopes is found to be $K_{\\tau} = -555 \\pm 75$ MeV, confirming the value previously obtained from the Sn isotopes. ISGMR strength has been computed in relativistic RPA using NL3 and FSUGold effective interactions. Both models significantly overestimate the centroids of the ISGMR strength in the Cd isotopes. Combined with other recent theoretical effort, the question of the "softness" of the open-shell nuclei in the tin region remains open still.

  20. Giant monopole resonance in even-A Cd isotopes, the asymmetry term in nuclear incompressibility, and the 'softness' of Sn and Cd nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Patel, D. [Department of Physics, University of Notre Dame, Notre Dame, IN 46556 (United States); Garg, U., E-mail: garg@nd.edu [Department of Physics, University of Notre Dame, Notre Dame, IN 46556 (United States); Fujiwara, M. [Research Center for Nuclear Physics, Osaka University, Osaka 567-0047 (Japan); Akimune, H. [Department of Physics, Konan University, Kobe 568-8501 (Japan); Berg, G.P.A. [Department of Physics, University of Notre Dame, Notre Dame, IN 46556 (United States); Harakeh, M.N. [Kernfysisch Versneller Instituut, University of Groningen, 9747 AA Groningen (Netherlands); Itoh, M. [Cyclotron and Radioisotope Center, Tohoku University, Sendai 980-8578 (Japan); Kawabata, T. [Center for Nuclear Studies, University of Tokyo, Tokyo 113-0033 (Japan); Kawase, K. [Institute of Scientific and Industrial Research, Osaka University, Osaka 567-0047 (Japan); Nayak, B.K. [Department of Physics, University of Notre Dame, Notre Dame, IN 46556 (United States); Ohta, T. [Research Center for Nuclear Physics, Osaka University, Osaka 567-0047 (Japan); Ouchi, H. [Cyclotron and Radioisotope Center, Tohoku University, Sendai 980-8578 (Japan); Piekarewicz, J. [Department of Physics, Florida State University, Tallahassee, FL 32306 (United States); Uchida, M. [Department of Physics, Tokyo Institute of Technology, Tokyo 152-8850 (Japan); Yoshida, H.P. [Cyclotron and Radioisotope Center, Tohoku University, Sendai 980-8578 (Japan); Yosoi, M. [Research Center for Nuclear Physics, Osaka University, Osaka 567-0047 (Japan)

    2012-12-05

    The isoscalar giant monopole resonance (ISGMR) in even-A Cd isotopes has been studied by inelastic {alpha}-scattering at 100 MeV/u and at extremely forward angles, including 0 Degree-Sign . The asymmetry term in the nuclear incompressibility extracted from the ISGMR in Cd isotopes is found to be K{sub {tau}}=-555{+-}75 MeV, confirming the value previously obtained from the Sn isotopes. ISGMR strength has been computed in relativistic RPA using NL3 and FSUGold effective interactions. Both models significantly overestimate the centroids of the ISGMR strength in the Cd isotopes. Combined with other recent theoretical effort, the question of the 'softness' of the open-shell nuclei in the tin region remains open still.

  1. N3LO NN interaction adjusted to light nuclei in ab exitu approach

    Science.gov (United States)

    Shirokov, A. M.; Shin, I. J.; Kim, Y.; Sosonkina, M.; Maris, P.; Vary, J. P.

    2016-10-01

    We use phase-equivalent transformations to adjust off-shell properties of similarity renormalization group evolved chiral effective field theory NN interaction (Idaho N3LO) to fit selected binding energies and spectra of light nuclei in an ab exitu approach. We then test the transformed interaction on a set of additional observables in light nuclei to verify that it provides reasonable descriptions of these observables with an apparent reduced need for three- and many-nucleon interactions.

  2. 补强圈与筒体间隙对开孔补强结构强度的影响%Influence of the Gap between Reinforcement Pad and Shell on the Structural Strength of Opening Reinforcement

    Institute of Scientific and Technical Information of China (English)

    李岩; 杨世明

    2016-01-01

    在评定压力容器开孔补强结构强度时,经典薄壳理论未考虑补强圈与筒体间隙,而间隙却在实际结构中存在。设筒体承受不同的内压值、接管上承受不同的轴向力,应用有限元软件的接触算法对压力容器开孔补强结构进行了静强度与疲劳强度评定,考察了不同间隙值对强度的影响,同时也计算了未考虑接触时的结果作为对比。结果分析表明:在接管有正向轴向力存在的情况下有必要考虑接触,而补强圈与筒体之间间隙大小在评定开孔补强结构静强度与由内压或者轴向变载引起的疲劳强度时的影响可以忽略。%When evaluating the strength of the opening reinforcement structure of pressure vessels, the classical thin shell the-ory doesn't take into account the interstice between the reinforcement structure rings and cylinder, but in fact, the interstice exists in the structure.The opening reinforcement structure of pressure vessels with different pressure values on the cylinder and different axial force values on nozzle are computed by the contact algorithm of ANSYS in order to evaluate the static strength and fatigue strength.Besides, the influence of different interstices on strength is examined, and the comparison be-tween the results of with the contact and without the contact is made.The results show that the gap between the reinforcement structure rings and cylinder should be considered in the case of the nozzle with positive axial force, while the influence of the interstice size can be ignored when evaluating the opening reinforcement structure of pressure vessels static strength and the fa-tigue strength of only internal pressure or the extra axial force on nozzle.

  3. Interplay between one-particle and collective degrees of freedom in nuclei

    CERN Document Server

    Hamamoto, Ikuko

    2016-01-01

    Some developments of nuclear-structure physics uniquely related to Copenhagen School are sketched based on theoretical considerations versus experimental findings and one-particle versus collective aspects. Based on my personal overview I pick up the following topics; (1) Study of vibration in terms of particle-vibration coupling; (2) One-particle motion in deformed and rotating potentials, and yrast spectroscopy in high-spin physics; (3) Triaxial shape in nuclei: wobbling motion and chiral bands; (4) Nuclear structure of drip line nuclei: in particular, shell-structure (or magic numbers) change and spherical or deformed halo phenomena; (5) shell structure in oblate deformation.

  4. Structure of the N=50 As, Ge, Ga nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Sahin, E., E-mail: eda.sahin@lnl.infn.it [Laboratori Nazionali di Legnaro dell' INFN, Legnaro (Italy); Department of Physics, University of Oslo, NO-0316 Oslo (Norway); Angelis, G. de [Laboratori Nazionali di Legnaro dell' INFN, Legnaro (Italy); Duchene, G.; Faul, T. [IPHC, IN2P3/CNRS et Universite Louis Pasteur, Strasbourg (France); Gadea, A. [Laboratori Nazionali di Legnaro dell' INFN, Legnaro (Italy); Instituto de Fisica Corpuscular, CSIC - Universidad de Valencia, Valencia (Spain); Lisetskiy, A.F. [Department of Physics, University of Arizona, Tucson, AZ (United States); Ackermann, D. [Helmholtzzentrum fuer Schwerionenforschung (GSI), Darmstadt (Germany); Algora, A. [Instituto de Fisica Corpuscular, CSIC - Universidad de Valencia, Valencia (Spain); Institute of Nuclear Research, Debrecen (Hungary); Aydin, S. [Department of Physics, University of Aksaray, Aksaray (Turkey); INFN Sezione di Padova and Dipartimento di Fisica, Universita di Padova, Padova (Italy); Azaiez, F. [IPNO, IN2P3/CNRS et Universite Paris-Sud, Orsay (France); Bazzacco, D. [INFN Sezione di Padova and Dipartimento di Fisica, Universita di Padova, Padova (Italy); Benzoni, G. [INFN Sezione di Milano and Dipartimento di Fisica, Universita di Milano, Milano (Italy); Bostan, M. [Department of Physics, Istanbul University, Istanbul (Turkey); Byrski, T. [IPHC, IN2P3/CNRS et Universite Louis Pasteur, Strasbourg (France); Celikovic, I. [Vinca Institute of Nuclear Sciences, Belgrade (Serbia); Chapman, R. [University of the West of Scotland, Paisley (United Kingdom); Corradi, L. [Laboratori Nazionali di Legnaro dell' INFN, Legnaro (Italy); and others

    2012-11-02

    The level structures of the N=50{sup 83}As, {sup 82}Ge, and {sup 81}Ga isotones have been investigated by means of multi-nucleon transfer reactions. A first experiment was performed with the CLARA-PRISMA setup to identify these nuclei. A second experiment was carried out with the GASP array in order to deduce the {gamma}-ray coincidence information. The results obtained on the high-spin states of such nuclei are used to test the stability of the N=50 shell closure in the region of {sup 78}Ni (Z=28). The comparison of the experimental level schemes with the shell-model calculations yields an N=50 energy gap value of 4.7(3) MeV at Z=28. This value, in a good agreement with the prediction of the finite-range liquid-drop model as well as with the recent large-scale shell model calculations, does not support a weakening of the N=50 shell gap down to Z=28.

  5. Skyrmions and Nuclei

    Science.gov (United States)

    Battye, R. A.; Manton, N. S.; Sutcliffe, P. M.

    We review recent work on the modelling of atomic nuclei as quantised Skyrmions, using Skyrme's original model with pion fields only. Skyrmions are topological soliton solutions, whose conserved topological charge B is identified with the baryon number of a nucleus. Apart from an energy and length scale, the Skyrme model has just one dimensionless parameter m, proportional to the pion mass. It has been found that a good fit to experimental nuclear data requires m to be of order 1. The Skyrmions for B up to 7 have been known for some time, and are qualitatively insensitive to whether m is zero or of order 1. However, for baryon numbers B = 8 and above, the Skyrmions have quite a compact structure for m of order 1, rather than the hollow polyhedral structure found when m = 0. One finds for baryon numbers which are multiples of four, that the Skyrmions are composed of B = 4 sub-units, as in the α-particle model of nuclei. The rational map ansatz gives a useful approximation to the Skyrmion solutions for all baryon numbers when m = 0. For m of order 1, it gives a good approximation for baryon numbers up to 7, and generalisations of this ansatz are helpful for higher baryon numbers. We briefly review the work from the 1980s and 90s on the semiclassical rigidbody quantisation of Skyrmions for B = 1, 2, 3 and 4. We then discuss more recent work extending this method to B = 6, 7, 8, 10 and 12. We determine the quantum states of the Skyrmions, finding their spins, isospins and parities, and compare with the experimental data on the ground and excited states of nuclei up to mass number 12.

  6. Active galactic nuclei

    CERN Document Server

    Beckmann, Volker

    2012-01-01

    This AGN textbook includes phenomena based on new results in the X-Ray domain from new telescopes such as Chandra and XMM Newton not mentioned in any other book. Furthermore, it considers also the Fermi Gamma Ray Space Telescope with its revolutionary advances of unprecedented sensitivity, field of view and all-sky monitoring. Those and other new developments as well as simulations of AGN merging events and formations, enabled through latest super-computing capabilities. The book gives an overview on the current knowledge of the Active Galacitc Nuclei phenomenon. The spectral energy d

  7. Active galactic nuclei

    CERN Document Server

    Blandford, RD; Woltjer, L

    1990-01-01

    Starting with this volume, the Lecture Notes of the renowned Advanced Courses of the Swiss Society for Astrophysics and Astronomy will be published annually. In each course, three extensive lectures given by leading experts in their respective fields cover different and essential aspects of the subject. The 20th course, held at Les Diablerets in April 1990, dealt with current research on active galactic nuclei; it represents the most up-to-date views on the subject, presented with particular regard for clarity. The previous courses considered a wide variety of subjects, beginning with ""Theory

  8. Visibility of comet nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Ney, E.P.

    1982-01-22

    Photography of the nucleus of comet Halley is the goal of several planned space missions. The nucleus of a comet is surrounded by a cloud of dust particles. If this cloud is optically thick, it will prevent observation of the nuclear surface. Broadband photometry of nine comets has been analyzed to determine the visibility of their nuclei. Only in the case of comet West near perihelion was the dust dense enough to interfere with imaging. Comparison of the visual brightness of the well-observed comets with that of Halley in 1910 leads to the conclusion that the nucleus of Halley can be imaged without significant obscuration by the dust.

  9. Shape coexistence and shell evolution in the 68Ni region

    Science.gov (United States)

    Chiara, C. J.

    2016-09-01

    Studies of nuclei along or near the line of stability have long since demonstrated the existence of certain magic numbers of protons or neutrons, corresponding to shell closures where there are large energy gaps among the single-particle orbitals. Nuclei located near these magic numbers tend to have increased stability compared to their neighbors and are typically spherical in their ground states. As technological advances continue to push our reach to nuclei farther from stability, mounting evidence has revealed that this familiar shell structure changes with increasing asymmetry in the numbers of neutrons and protons. The disappearance of some well-known magic numbers and the formation of new ones, driven largely by the tensor force, have both been identified. Along with this shell evolution as a function of nucleon number, a different type can also occur within a given nucleus as a consequence of configuration changes and the corresponding effect of their associated nuclear forces. This latter type of shell evolution manifests itself as a coexistence of spherical and deformed shapes at low excitation energies. Highlights will be presented of recent research on shell evolution in neutron-rich nuclei in the vicinity of 68Ni. Particular emphasis will be given to the efforts at Argonne National Laboratory and the National Superconducting Cyclotron Laboratory which have revealed new structure in these nuclei through multinucleon-transfer reactions and beta-decay spectroscopy. These experimental results could only be explained by concurrent advances in the corresponding shell-model description, requiring larger model spaces than could previously be accommodated. Supported by the US Army Research Lab under Cooperative Agreement W911NF-12-2-0019.

  10. Statistical properties of quantum spectra in nuclei

    Institute of Scientific and Technical Information of China (English)

    WU; Xizhen

    2001-01-01

    [1]Wu Xizhen,Sakata,F.,Zhuo Yizhong et al.,Dynamic realization of statistical state in finite systems,Phys.ReV.C,1996,53:1233-1244.[2]Weidenmüller,H.A.,Statistical theory of nuclear reactions and the Gaussian Othogonal Ensemble,Annals of Physics,1984,158:120-141.[3]Hag,R.U.,Pandey,A.,Bohigas,O.,Fluctuation properties of nuclear energy levels:Do theory and experiment agree? Phys.Rev.Lett.,1982,48:1086-1089.[4]Wu Xizhen,Gu Jianzhong,Iwamoto,A.,Statistical properties of quasiparticle spectra in deformed nuclei,Phys.Rev.C,1999,59:215-220.[5]Garrett,J.D.,Robinson,J.Q.,Foglia,A.J.et al.,Nuclear level repulsion and order vs chaos,Phys.Lett.B,1997,392:24-29.[6]Bohigas,O.,Hag,R.U.,Pandy,A.,Fluctuation properties of nuclear energy levels and widths comparison of theory with experiment,in Nuclear Data for Science and Technology (ed.Bockhoff,K.H.),Dordrecht:Reidel,1983,809-813.[7]Heiss,W.D.,Nazmitdinov,R.G.,Radu,S.,Chaos in axially symmetric potentials with Octupole deformation,Phys.Rev.Lett.,1994,72:2351-2354.[8]Wu Xizhen,Gu Jianzhong,Zhuo Yizhong et al.,Possible understanding of hyperdeformed 144-146Ba nuclei appearing in the spontaneous fission of 252Cf,Phys.Rev.Lett.,1997,79:4542-4545.[9]Ter-Akopian,G.M.,Hamilton,J.H.,Oganessian,Y.T.et al.,New spontaneous fission mode for 252Cf:Indication of hyperdeformed 144,145,146Ba at scission,Phys.Rev.Lett.,1996,77:32-35.[10]Adamian,G.G.,Antonenko,N.V.,Ivanova,S.P.et al.,Problems in description of fusion of heavy nuclei in the two-center shell model approach,Nucl.Phys.A,1999,646:29-52.[11]Hofmann,H.,A quantal transport theory for nuclear collective motion:the metrits of a locally harmonic approximation method,Phys.Rep.,1997,284:139-380.[12]Gu Jianzhong,Wu Xizhen,Zhuo Yizhong,Quantum chaotic motion of a single particle in heavy nuclei,Nucl.Phys.A,1997,625:621-632.[13]Gu Jianzhong,Wu Xizhen,Zhuo Yizhong,The single-particle spectrum and its spacing and curvature distributions in

  11. Elusive Active Galactic Nuclei

    CERN Document Server

    Maiolino, R; Gilli, R; Nagar, N M; Bianchi, S; Böker, T; Colbert, E; Krabbe, A; Marconi, A; Matt, G; Salvati, M

    2003-01-01

    A fraction of active galactic nuclei do not show the classical Seyfert-type signatures in their optical spectra, i.e. they are optically "elusive". X-ray observations are an optimal tool to identify this class of objects. We combine new Chandra observations with archival X-ray data in order to obtain a first estimate of the fraction of elusive AGN in local galaxies and to constrain their nature. Our results suggest that elusive AGN have a local density comparable to or even higher than optically classified Seyfert nuclei. Most elusive AGN are heavily absorbed in the X-rays, with gas column densities exceeding 10^24 cm^-2, suggesting that their peculiar nature is associated with obscuration. It is likely that in elusive AGN, the nuclear UV source is completely embedded and the ionizing photons cannot escape, which prevents the formation of a classical Narrow Line Region. Elusive AGN may contribute significantly to the 30 keV bump of the X-ray background.

  12. Spurious Shell Closures in the Relativistic Mean Field Model

    CERN Document Server

    Geng, L S; Toki, H; Long, W H; Shen, G

    2006-01-01

    Following a systematic theoretical study of the ground-state properties of over 7000 nuclei from the proton drip line to the neutron drip line in the relativistic mean field model [Prog. Theor. Phys. 113 (2005) 785], which is in fair agreement with existing experimental data, we observe a few spurious shell closures, i.e. proton shell closures at Z=58 and Z=92. These spurious shell closures are found to persist in all the effective forces of the relativistic mean field model, e.g. TMA, NL3, PKDD and DD-ME2.

  13. Electron scattering for exotic nuclei

    Indian Academy of Sciences (India)

    Toshimi Suda

    2014-11-01

    A brand-new electron scattering facility, the SCRIT Electron Scattering Facility, will soon start its operation at RIKEN RI Beam Factory, Japan. This is the world’s first electron scattering facility dedicated to the structure studies of short-lived nuclei. The goal of this facility is to determine the charge density distributions of short-lived exotic nuclei by elastic electron scattering. The first collision between electrons and exotic nuclei will be observed in the year 2014.

  14. Evaluation of Coulomb Energy Difference for Light Mirror Nuclei Using Slater—Type Orbitals

    Institute of Scientific and Technical Information of China (English)

    F.Oner; R.A.Mamedoy

    2002-01-01

    Behavior of the Coulomb energy difference for light nuclei is explained in terms of the different values of the average Coulomb interaction between two particles.Coulomb energy difference according to shell model of light mirror nuclei in the Coulomb and exchange integrals in the formula can be explained with exponential-type wavefunctions.In this study,using the one-center expansion of exponential-type wavefunctions in terms of Slater-type orbitals with the same center,we derived formula for Coulomb energy difference of light mirror nuclei.

  15. A Statistical Approach to Describe Highly Excited Heavy and Superheavy Nuclei

    CERN Document Server

    Chen, Peng-Hui; Li, Jun-Qing; Zhang, Hong-Fei

    2016-01-01

    A statistical approach based on the Weisskopf evaporation theory has been developed to describe the de-excitation process of highly excited heavy and superheavy nuclei, in particular for the proton-rich nuclei. The excited nucleus is cooled by evaporating $\\gamma$-ray, light particles (neutrons, protons, $\\alpha$ etc) in competition with the binary fission, in which the structure effects (shell correction, fission barrier, particle separation energy) contribute to the processes. The formation of residual nuclei is evaluated via sequential emission of possible particles above the separation energies. The available data of fusion-evaporation excitation functions in the $^{28}$Si+$^{198}$Pt reaction can be reproduced nicely well within the approach.

  16. Shell Analysis Manual

    Science.gov (United States)

    1968-04-01

    loading (e. g. shallow shell theory , Geckeler’s approximation for symmetrically loaded shells, etc.) Although the Shear Deformation and Specialized...interest. Included are the Reissner-Meissner equations, Geckeler’s approximations, shallow - shell theory , Donnell’s theory, and others. A. General Shells of

  17. Superheavy nuclei: from predictions to discovery

    Science.gov (United States)

    Oganessian, Yu Ts; Sobiczewski, A.; Ter-Akopian, G. M.

    2017-02-01

    A fundamental outcome of modern nuclear microscopic theory is the prediction of the ‘islands of stability’ in the region of hypothetical superheavy elements (SHEs). In a heavy nucleus, going through the large-scale deformation on the way to fission, the motion of single nucleons is coupled with the collective degrees of freedom of the whole system. The most striking effect of this coupling is obtained for the case of fission of the heaviest nuclei, whose existence is defined entirely by the nuclear structure, i.e. by the shell effect. From this point of view, the synthesis and study of properties of superheavy nuclei (SHN) is a direct way for checking the basic statements of the microscopic nuclear theory. On the nuclide map, SHN outline the border of the heaviest nuclear masses. SHN set the limits of the periodic system of chemical elements. The study of possible existence of SHN in nature offers a way for testing different scenarios of astrophysical nucleosynthesis. The paper elucidates experimental approaches, used for testing the theory predictions made about the SHN, and presents the results of the discovery of the ‘stability island’ of SHEs.

  18. Chemical complexity in galactic nuclei

    Science.gov (United States)

    Martin-Pintado, Jesus

    2007-12-01

    In recent years our knowledge of the chemical complexity in the nuclei of galaxies has dramatically changed. Recent observations of the nucleus of the Milky Way, of the starburst galaxy NGC253 and of the ultraluminous infrared galaxy (ULIRG) Arp220 have shown large abundance of complex organic molecules believed to be formed on grains. The Galactic center appears to be the largest repository of complex organic molecule like aldehydes and alcohols in the galaxy. We also measure large abundance of methanol in starburst galaxies and in ULIRGs suggesting that complex organic molecules are also efficiently produced in the central region of galaxies with strong star formation activity. From the systematic observational studies of molecular abundance in regions dominated by different heating processes like shocks, UV radiation, X-rays and cosmic rays in the center of the Milky Way, we are opening the possibility of using chemistry as a diagnostic tool to study the highly obscured regions of galactic centers. The templates found in the nucleus of the Milky Way will be used to establish the main mechanisms driving the heating and the chemistry of the molecular clouds in galaxies with different type of activity. The role of grain chemistry in the chemical complexity observed in the center of galaxies will be also briefly discussed.

  19. Dynamic Properties of Viscoelastic Open Shallow Shells

    Institute of Scientific and Technical Information of China (English)

    2000-01-01

    1 Introduction Totheauthors’knowledge ,therearerarelypapersconcerningthedynamicbehaviorofviscoelasticshells.Uptonowmostofworkwasconcernedwiththestabilityofviscoelasticshells.Potapov ( 1978) [1]studiedthestabilityofcompressedviscoelasticor thotropicshells.DingR .( 1997) [2 ] discussedthedy namicbehaviorofviscoelasticshellswithsmalldeflec tionsandobtainedsomemeaningfulresults . Inthis paper ,basedonthehypothesesoftheK偄rm偄n Donnelltheoryofthinshellswithlargede flectionsandtheBoltzmannlawsforlinearviscoelasticm...

  20. Global systematics of unique parity quasibands in odd-[ital A] collective nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Bucurescu, D.; Cata-Danil, G.; Ivascu, M.; Stroe, L.; Ur, C.A. (Institute of Atomic Physics, P.O. Box MG-6, Bucharest (Romania))

    1994-04-01

    All known structures in the collective medium and heavy odd-[ital A] nuclei, based on the unique parity orbitals [ital g][sub 9/2], [ital h][sub 11/2], and [ital i][sub 13/2], are collected and correlations between the energies within both the favored and unfavored quasibands are analyzed. A first startling result is that irrespective of the nature of the odd particle and the shell model orbital, for most of the nondeformed nuclei the energies within these quasibands, show a universal behavior of an anharmonic vibrator with a constant anharmonicity, identical with that found for the even-even nuclei. Second, the rapid transition between the anharmonic vibrator and the rotor regimes, which takes place in the even-even nuclei, is accompanied, in the adjacent odd-[ital A] nuclei, by an equally rapid transition from the anharmonic vibrator to the strong coupling regime.

  1. PREFACE: Structure of Exotic Nuclei and Nuclear Forces

    Science.gov (United States)

    Honma, Michio; Otsuka, Takaharu; Aoi, Nori

    2006-11-01

    The International Symposium on `Structure of Exotic Nuclei and Nuclear Forces' was held at The Koshiba Hall, University of Tokyo, on 9 - 12 March 2006. This symposium was organized as an activity of the Grant-in-Aid for the specially promoted area `Monte Carlo Shell Model' from the Ministry of Education, Science, Sports and Culture (MEXT) of Japan. The symposium was sponsored by the Center for Nuclear Study (CNS) and by RIKEN. The purpose of the symposium was to discuss theoretical and experimental developments in the study of the structure of exotic nuclei and its relationship with nuclear forces. There has been much progress recently in our understanding of what the structure of exotic nuclei is and how it can be linked to nuclear forces, with emerging intriguing perspectives. The following subjects were covered in this symposium Present status and future of the shell model Effective interaction theories Experimental results and perspectives Few-body methods including ab initio calculations Advancements of mean-fieeld models Transition between shell and cluster structure Nuclear astrophysics and nuclear structure Particle physics and the shell model Emphasis was placed on the interplay between many-body structures and nuclear forces, and on the experimental clarification of these topics. Around 80 participants attended the symposium and we enjoyed 34 excellent and lively invited talks and 26 oral presentations. The organizing committee consisted of B A Brown (MSU), S Fujii (CNS), M Honma (Aizu), T Kajino (NAO), T Mizusaki (Senshu), T Motobayashi (RIKEN), K Muto (TIT), T Otsuka (Chair, Tokyo/CNS/RIKEN), P Ring (TMU), N Shimizu (Scientific Secretary, Tokyo), S Shimoura (CNS), Y Utsuno (Scientific Secretary, JAEA). Finally, we would like to thank all the speakers and the participants as well as the other organizers for their contributions which made the symposium so successful.

  2. The No-Core Gamow Shell Model: Including the continuum in the NCSM

    CERN Document Server

    Barrett, B R; Michel, N; Płoszajczak, M

    2015-01-01

    We are witnessing an era of intense experimental efforts that will provide information about the properties of nuclei far from the line of stability, regarding resonant and scattering states as well as (weakly) bound states. This talk describes our formalism for including these necessary ingredients into the No-Core Shell Model by using the Gamow Shell Model approach. Applications of this new approach, known as the No-Core Gamow Shell Model, both to benchmark cases as well as to unstable nuclei will be given.

  3. Clusters in nuclei

    CERN Document Server

    Following the pioneering discovery of alpha clustering and of molecular resonances, the field of nuclear clustering is today one of those domains of heavy-ion nuclear physics that faces the greatest challenges, yet also contains the greatest opportunities. After many summer schools and workshops, in particular over the last decade, the community of nuclear molecular physicists has decided to collaborate in producing a comprehensive collection of lectures and tutorial reviews covering the field. This third volume follows the successful Lect. Notes Phys. 818 (Vol. 1) and 848 (Vol. 2), and comprises six extensive lectures covering the following topics:  - Gamma Rays and Molecular Structure - Faddeev Equation Approach for Three Cluster Nuclear Reactions - Tomography of the Cluster Structure of Light Nuclei Via Relativistic Dissociation - Clustering Effects Within the Dinuclear Model : From Light to Hyper-heavy Molecules in Dynamical Mean-field Approach - Clusterization in Ternary Fission - Clusters in Light N...

  4. Gluon density in nuclei

    CERN Document Server

    Ayala, A P; Levin, E M

    1996-01-01

    In this talk we present our detail study ( theory and numbers) [1] on the shadowing corrections to the gluon structure functions for nuclei. Starting from rather contraversial information on the nucleon structure function which is originated by the recent HERA data, we develop the Glauber approach for the gluon density in a nucleus based on Mueller formula [2] and estimate the value of the shadowing corrections in this case. Than we calculate the first corrections to the Glauber approach and show that these corrections are big. Based on this practical observation we suggest the new evolution equation which takes into account the shadowing corrections and solve it. We hope to convince you that the new evolution equation gives a good theoretical tool to treat the shadowing corrections for the gluons density in a nucleus and, therefore, it is able to provide the theoretically reliable initial conditions for the time evolution of the nucleus - nucleus cascade.

  5. Pulsars: Gigantic Nuclei

    CERN Document Server

    Xu, Renxin

    2011-01-01

    What is the real nature of pulsars? This is essentially a question of the fundamental strong interaction between quarks at low-energy scale and hence of the non-perturbative quantum chromo-dynamics, the solution of which would certainly be meaningful for us to understand one of the seven millennium prize problems (i.e., "Yang-Mills Theory") named by the Clay Mathematical Institute. After a historical note, it is argued here that a pulsar is very similar to an extremely big nucleus, but is a little bit different from the {\\em gigantic nucleus} speculated 80 years ago by L. Landau. The paper demonstrates the similarity between pulsars and gigantic nuclei from both points of view: the different manifestations of compact stars and the general behavior of the strong interaction.

  6. Nucleomorphs: enslaved algal nuclei.

    Science.gov (United States)

    Cavalier-Smith, T

    2002-12-01

    Nucleomorphs of cryptomonad and chlorarachnean algae are the relict, miniaturised nuclei of formerly independent red and green algae enslaved by separate eukaryote hosts over 500 million years ago. The complete 551 kb genome sequence of a cryptomonad nucleomorph confirms that cryptomonads are eukaryote-eukaryote chimeras and greatly illuminates the symbiogenetic event that created the kingdom Chromista and their alveolate protozoan sisters. Nucleomorph membranes may, like plasma membranes, be more enduring after secondary symbiogenesis than are their genomes. Partial sequences of chlorarachnean nucleomorphs indicate that genomic streamlining is limited by the mutational difficulty of removing useless introns. Nucleomorph miniaturisation emphasises that selection can dramatically reduce eukaryote genome size and eliminate most non-functional nuclear non-coding DNA. Given the differential scaling of nuclear and nucleomorph genomes with cell size, it follows that most non-coding nuclear DNA must have a bulk-sequence-independent function related to cell volume.

  7. Review of alpha-decay data from doubly-even nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Akovali, Y.A.

    1996-09-01

    Alpha-decay data from doubly-even nuclei throughout the periodic table are reviewed and evaluated. From these data, nuclear radius parameters are calculated by using the Preston formula for {alpha}- decay probabilities. The radius parameters for each element behave rather regularly as a function of neutron number. The show minima at the major closed shells, increase sharply for parents just above the closed shells, and decrease smoothly toward the next shell closure. The same trend is observed for {alpha} reduced widths calculated using the Rasmussen formalism. Any irregularity or large departure from this behavior indicates probable incorrect input data. This systematic behavior can also be utilized to estimate partial half- lives.

  8. Self-consistent study of nuclei far from stability with the energy density method

    CERN Document Server

    Tondeur, F

    1981-01-01

    The self-consistent energy density method has been shown to give good results with a small number of parameters for the calculation of nuclear masses, radii, deformations, neutron skins, shell and sub- shell effects. It is here used to study the properties of nuclei far from stability, like densities, shell structure, even-odd mass differences, single-particle potentials and nuclear deformations. A few possible consequences of the results for astrophysical problems are briefly considered. The predictions of the model in the super- heavy region are summarised. (34 refs).

  9. Quarks in Few Body Nuclei

    Science.gov (United States)

    Holt, Roy J.

    2016-03-01

    Electron scattering at very high Bjorken x from hadrons provides an excellent test of models, has an important role in high energy physics, and from nuclei, provides a window into short range correlations. Light nuclei have a key role because of the relatively well-known nuclear structure. The development of a novel tritium target for Jefferson Lab has led to renewed interest in the mass three system. For example, deep inelastic scattering experiments in the light nuclei provide a powerful means to determine the neutron structure function. The isospin dependence of electron scattering from mass-3 nuclei provide information on short range correlations in nuclei. The program using the new tritium target will be presented along with a summary of other experiments aimed at revealing the large-x structure of the nucleon.

  10. Quarks in Few Body Nuclei

    Directory of Open Access Journals (Sweden)

    Holt Roy J.

    2016-01-01

    Full Text Available Electron scattering at very high Bjorken x from hadrons provides an excellent test of models, has an important role in high energy physics, and from nuclei, provides a window into short range correlations. Light nuclei have a key role because of the relatively well-known nuclear structure. The development of a novel tritium target for Jefferson Lab has led to renewed interest in the mass three system. For example, deep inelastic scattering experiments in the light nuclei provide a powerful means to determine the neutron structure function. The isospin dependence of electron scattering from mass-3 nuclei provide information on short range correlations in nuclei. The program using the new tritium target will be presented along with a summary of other experiments aimed at revealing the large-x structure of the nucleon.

  11. Cavitation inception from bubble nuclei

    DEFF Research Database (Denmark)

    Mørch, Knud Aage

    2015-01-01

    , and experimental investigations of bubbles and cavitation inception have been presented. These results suggest that cavitation nuclei in equilibrium are gaseous voids in the water, stabilized by a skin which allows diffusion balance between gas inside the void and gas in solution in the surrounding liquid....... The cavitation nuclei may be free gas bubbles in the bulk of water, or interfacial gaseous voids located on the surface of particles in the water, or on bounding walls. The tensile strength of these nuclei depends not only on the water quality but also on the pressure-time history of the water. A recent model......The tensile strength of ordinary water such as tap water or seawater is typically well below 1 bar. It is governed by cavitation nuclei in the water, not by the tensile strength of the water itself, which is extremely high. Different models of the nuclei have been suggested over the years...

  12. Nucleus-nucleus potential with shell-correction contribution

    CERN Document Server

    Denisov, V Yu

    2015-01-01

    The full relaxed-density potential between spherical nuclei is considered as a sum of the macroscopic and shell-correction contributions. The macroscopic part of the potential is related to a nucleus-nucleus potential obtained in the framework of the extended Thomas-Fermi approach with the Skyrme and Coulomb forces and the relaxed-density ansatz for evaluation of proton and neutron densities of interacting nuclei. A simple prescription for the shell-correction part of the total potential is discussed. The parameters of the shell-correction and macroscopic parts of the relaxed-density potential are found by fitting the empirical barrier heights of the 89 nucleus-nucleus systems as well as macroscopic potentials evaluated for 1485 nucleus-nucleus systems at 12 distances around touching points.

  13. Multiple shells in IRC+10216: shell properties

    Science.gov (United States)

    Mauron, N.; Huggins, P. J.

    2000-07-01

    We report on the properties of the multiple shells in the circumstellar envelope of IRC+10216, using deep optical imaging, including data from the Hubble Space Telescope. The intensity profiles confirm the presence of thin ( ~ 0farcs5 -3'' ec), limb-brightened shells in the envelope, seen in stellar and ambient Galactic light scattered by dust. The shells are spaced at irregular intervals of ~ 5'' ec-20'' ec, corresponding to time scales of 200-800 yr, although intervals as short as ~ 1'' ec (40 yr) are seen close to the star. The location of the main shells shows a good correlation with high-resolution, molecular line maps of the inner envelope, indicating that the dust and gas are well coupled. The shell/intershell density contrast is typically ~ 3, and we find that the shells form the dominant mass component of the circumstellar envelope. The shells exhibit important evolutionary effects: the thickness increases with increasing radius, with an effective dispersion velocity of 0.7 km s-1 and there is evidence for shell interactions. Despite the presence of bipolar structure close to the star, the global shell pattern favors a roughly isotropic, episodic mass loss mechanism, with a range of time scales. Based on observations made with the Canada-France-Hawaii telescope, operated by CNRS, NRCC and UH, and on dearchived observations made with the NASA/ESA Hubble Space Telescope, operated by AURA Inc., under NASA contract NAS5-26555

  14. Structure of negative parity yrast bands in odd mass 125-131Ce nuclei

    Indian Academy of Sciences (India)

    Arun Bharti; Suram Singh; S K Khosa

    2010-04-01

    The negative parity yrast bands of neutron-deficient 125-131Ce nuclei are studied by using the projected shell model approach. Energy levels, transition energies and (1)/(2) ratios are calculated and compared with the available experimental data. The calculations reproduce the band-head spins of negative parity yrast bands and indicate the multi-quasiparticle structure for these bands.

  15. Skyrme–Hartree–Fock approach to the change of level occupancy of low mass halo nuclei

    Indian Academy of Sciences (India)

    Rupayan Bhattacharya

    2000-02-01

    With a new parameterization of potential parameters which reproduces the ground state properties of shell closed nuclei fairly accurately, the role of occupancy of 21/2 level in determining the halo structures of 17O, 16N, 15C, 14B, 13Be have been investigated. The results show interesting cross over of level occupancies which may explain the increase in interaction radii.

  16. Deformed pseudospin doublets as a fingerprint of a relativistic supersymmetry in nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Leviatan, A, E-mail: ami@phys.huji.ac.il [Racah Institute of Physics, The Hebrew University, Jerusalem 91904 (Israel)

    2011-01-01

    The single-particle spectrum of deformed shell-model states in nuclei, is shown to exhibit a supersymmetric pattern. The latter involves deformed pseudospin doublets and intruder levels. The underlying supersymmetry is associated with the relativistic pseudospin symmetry of the nuclear mean-field Dirac Hamiltonian with scalar and vector potentials.

  17. Deformed Pseudospin Doublets as a Fingerprint of a Relativistic Supersymmetry in Nuclei

    CERN Document Server

    Leviatan, A

    2010-01-01

    The single-particle spectrum of deformed shell-model states in nuclei, is shown to exhibit a supersymmetric pattern. The latter involves deformed pseudospin doublets and intruder levels. The underlying supersymmetry is associated with the relativistic pseudospin symmetry of the nuclear mean-field Dirac Hamiltonian with scalar and vector potentials.

  18. Decay properties of nuclei close to Z = 108 and N = 162

    Energy Technology Data Exchange (ETDEWEB)

    Dvorak, Jan

    2007-07-12

    The goal of the research conducted in the frame of this thesis was to investigate the decay properties of the nuclides {sup 269-271}Hs and their daughters using an improved chemical separation and detection system. Shell stabilization was predicted in the region around Z=108 and N=162 in calculations, taking into account possible higher orders of deformations of the nuclei. The nucleus {sup 270}Hs with a closed proton and a closed neutron deformed shell, was predicted to be ''deformed doubly magic''. Nuclei around {sup 270}Hs can be produced only via fusion reactions at picobarn levels, resulting in a production rates of few atoms per day. Investigating short-lived nuclei using rapid chemical separation and subsequent on-line detection methods provides an independent and alternative means to electromagnetic on-line separators. Chemical separation of Hs in the form of HsO{sub 4} provides an excellent tool to study the formation reactions and nuclear structure in this region of the chart of nuclides due to a high overall efficiency and a very high purification factor. The goal was accomplished, as element 108, hassium, was produced in the reaction {sup 248}Cm({sup 26}Mg,xn){sup 274-x}Hs and chemically isolated. After gas phase separation of HsO{sub 4}, 26 genetically linked decay chains have been observed. These were attributed to decays of three different Hs isotopes produced in the 3-5n evaporation channels. The known decay chain of {sup 269}Hs, the 5n evaporation product, serves as an anchor point, thus allowing the unambiguous assignment of the observed decay chains to the 5n, 4n, and 3n channels, respectively. Decay properties of five nuclei have been unambiguously established for the first time, including the one for the the doubly-magic nuclide {sup 270}Hs. This hassium isotope is the next doubly magic nucleus after the well known {sup 208}Pb and the first experimentally observed even-even nucleus on the predicted N=162 neutron shell. The

  19. Cavitation nuclei in water exposed to transient pressures

    DEFF Research Database (Denmark)

    Andersen, Anders Peter; Mørch, Knud Aage

    2015-01-01

    A model of skin-stabilized interfacial cavitation nuclei and their response to tensile and compressive stressing is presented. The model is evaluated in relation to experimental tensile strength results for water at rest at the bottom of an open water-filled container at atmospheric pressure and ...

  20. From super-charged nuclei to massive nuclear density cores

    CERN Document Server

    Popov, Vladimir

    2010-01-01

    Due to $e^+e^-$-pair production in the field of supercritical $(Z \\gg Z_{cr}\\approx 170 $) nucleus an electron shell, created out of the vacuum, is formed. The distribution of the vacuum charge in this shell has been determined for super-charged nuclei $Ze^3 \\ga 1$ within the framework of the Thomas-Fermi equation generalized to the relativistic case. For $Ze^3 \\gg 1$ the electron shell penetrates inside the nucleus and almost completely screens its charge. Inside such nucleus the potential takes a constant value equal to $V_0=-(3\\pi^2 n_p)^{1/3} \\sim -2m_{\\pi}c^2$, and super-charged nucleus represents an electrically neutral plasma consisting of $e,p$ and $n$. Near the edge of the nucleus a transition layer exists with a width $\\lambda \\approx \\alpha^{-1/2} \\hbar/m_{\\pi} c\\sim 15$ fm, which is independent of $Z~~ (\\hbar/m_{\\pi} c \\ll \\lambda \\ll \\hbar/m_e c)$. The electric field and surface charge are concentrated in this layer. These results, obtained earlier for hypothetical superheavy nuclei with $Z \\sim ...

  1. The cochlear nuclei of snakes.

    Science.gov (United States)

    Miller, M R

    1980-08-15

    The cochlear nuclei of three burrowing snakes (Xenopeltis unicolor, Cylindrophis rufus, and Eryx johni) and three non-burrowing snakes (Epicrates cenchris, Natrix sipedon, and Pituophis catenifer) were studied. The posterior branch of the statoacoustic nerve and its posterior ganglion were destroyed and the degenerated nerve fibers and terminals traced to primary cochlear nuclei in 13 specimens of Pituophis catenifer. All these snake species possess three primary and one secondary cochlear nuclei. The primary cochlear nuclei consist of a small nucleus angularis located at the cerebello-medullary junction and a fairly large nucleus magnocellularis forming a dorsal cap over the cephalic end of the alar eminence. Nucleus magnocellularis may be subdivided into a medially placed group of rounder cells, nucleus magnocellularis medialis, and a laterally placed group of more ovate and paler-staining cells, nucleus magnocellularis lateralis. A small but well-defined secondary nucleus which showed no degenerated nerve terminals after nerve root section, nucleus laminaris, underlies the cephalic part of both nucleus magnocellularis medialis and nucleus magnocellularis lateralis. Larger and better-developed cochlear nuclei were found in burrowing species than in non-burrowing species of snakes. Of the three burrowing species studied, Xenopeltis showed the greatest development of cochlear nuclei; Eryx cochlear nuclei were not quite as large but were better differentiated than in Xenopeltis; and Cylindrophis cochlear nuclei were fairly large but not as well developed nor as well differentiated as in either Xenopeltis or Eryx. The cochlear nuclei of the three non-burrowing snakes, Epicrates, Natrix, and Pituophis, were not as large nor as well developed as those of the burrowing snakes. There is some, but not complete, correlation between cochlear development and papilla basilaris length and number of hair cells. Thus, Xenopeltis and Eryx, with well-developed cochlear nuclei

  2. Exotic nuclei: another aspect of nuclear structure; Les noyaux exotiques: un autre regard sur la structure nucleaire

    Energy Technology Data Exchange (ETDEWEB)

    Dobaczewski, J. [Warsaw Univ., Institute of Theoretical Physics (Poland); Blumenfeld, Y.; Flocard, H.; Garcia Borge, M.J.; Nowacki, F.; Rombouts, S.; Theisen, Ch.; Marques, F.M.; Lacroix, D.; Dessagne, P.; Gaeggeler, H

    2002-07-01

    This document gathers the lectures made at the Joliot Curie international summer school in 2002 whose theme that year was exotic nuclei. There were 11 contributions whose titles are: 1) interactions, symmetry breaking and effective fields from quarks to nuclei; 2) status and perspectives for the study of exotic nuclei: experimental aspects; 3) the pairing interaction and the N = Z nuclei; 4) borders of stability region and exotic decays; 5) shell structure of nuclei: from stability to decay; 6) variational approach of system with a few nucleons; 7) from heavy to super-heavy nuclei; 8) halos, molecules and multi-neutrons; 9) macroscopic approaches for fusion reactions; 10) beta decay: a tool for spectroscopy; 11) the gas phase chemistry of super-heavy elements.

  3. Collective excitations in nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Chomaz, Ph

    1997-12-31

    The properties of the nucleus cannot be reduced to the properties of its constituents: it is a complex system. The fact that many properties of the nucleus are consequences of the existence of mean-field potential is a manifestation of this complexity. In particular the nucleons can thus self-organize in collective motions such as giant resonances. Therefore the study of these collective motions is a very good to understand the properties of the nucleus itself. The purpose of this article was to stress some aspects of these collective vibrations. In particular we have studied how an ensemble of fermions as the nucleus can self-organize in collective vibrations which are behaving like a gas of bosons in weak interaction. The understanding of these phenomena remains one of the important subjects of actually in the context of quantal systems in strong interaction. In particular the study of the states with one or two vibration quanta provides a direct information on the structure if nuclei close to their ground states. (author) 270 refs.

  4. Gluon density in nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Ayala, A.L. [Rio Grande do Sul Univ., Porto Alegre, RS (Brazil). Inst. de Fisica][Pelotas Univ., RS (Brazil). Inst. de Fisica e Matematica; Ducati, M.B.G. [Rio Grande do Sul Univ., Porto Alegre, RS (Brazil). Inst. de Fisica; Levin, E.M. [Fermi National Accelerator Lab., Batavia, IL (United States)][Nuclear Physics Inst., St. Petersburg (Russian Federation)

    1996-10-01

    In this talk we present our detailed study (theory and numbers) on the shadowing corrections to the gluon structure functions for nuclei. Starting from rather controversial information on the nucleon structure function which is originated by the recent HERA data, we develop the Glauber approach for the gluon density in a nucleus based on Mueller formula and estimate the value of the shadowing corrections in this case. Then we calculate the first corrections to the Glauber approach and show that these corrections are big. Based on this practical observation we suggest the new evolution equation which takes into account the shadowing corrections and solve it. We hope to convince you that the new evolution equation gives a good theoretical tool to treat the shadowing corrections for the gluons density in a nucleus and, therefore, it is able to provide the theoretically reliable initial conditions for the time evolution of the nucleus-nucleus cascade. The initial conditions should be fixed both theoretically and phenomenologically before to attack such complicated problems as the mixture of hard and soft processes in nucleus-nucleus interactions at high energy or the theoretically reliable approach to hadron or/and parton cascades for high energy nucleus-nucleus interaction. 35 refs., 24 figs., 1 tab.

  5. Monopole transitions in hot nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Sujkowski, Z. [Soltan Inst. for Nuclear Studies, Otwock-Swierk (Poland)

    1994-12-31

    Monopole transitions can be a signature of shape changing in a hot, pulsating nucleus (the low energy E0 mode) and/or a measure of the compressibility of finite nuclei (GMR, the breathing mode). Experimental information pertaining to GMR is reviewed. Recipes for deducing the incompressibility modules for infinite nuclear matter from data on GMR are discussed. Astrophysical implications are outlined. The first attempts at locating the GMR strength in moderately hot nuclei are described. Prospects for improving the experimental techniques to make an observation of this strength in selected nuclei unambiguous are discussed. (author). 46 refs, 8 figs.

  6. Spectroscopy of heavy fissionable nuclei

    Indian Academy of Sciences (India)

    S K Tandel

    2015-09-01

    Structural studies of heavy nuclei are quite challenging due to increased competition from fission, particularly at high spins. Nuclei in the actinide region exhibit a variety of interesting phenomena. Recent advances in instrumentation and analysis techniques have made feasible sensitive measurements of nuclei populated with quite low cross-sections. These include isomers and rotational band structures in isotopes of Pu ( = 94) to Rf ( = 104), and octupole correlations in the Th ( = 90) region. The obtained experimental data have provided insights on various aspects like moments of inertia and nucleon alignments at high spins, quasiparticle energies and evolution of quadrupole and octupole collectivity, among others. An overview of some of these results is presented.

  7. Probable alpha and $14$^C cluster emission from hyper Ac nuclei

    CERN Document Server

    Santhosh, K P

    2013-01-01

    A systematic study on the probability for the emission of 4^He and 14^C cluster from hyper ${207-234}^$Ac and non-strange normal ${207-234}^$Ac nuclei are performed for the first time using our fission model, the Coulomb and proximity potential model (CPPM). The predicted half lives show that hyper ${207-234}^$Ac nuclei are unstable against 4^He emission and 14^C emission from hyper ${217-228}^$Ac are favorable for measurement. Our study also show that hyper ${207-234}^$Ac are stable against hyper 4^He and 14^C emission. The role of neutron shell closure (N=126) in hyper 214^Fr daughter and role of proton/ neutron shell closure (Z =82, N =126) in hyper 210^Bi daughter are also revealed. As hyper-nuclei decays to normal nuclei by mesonic/non-mesonic decay and since most of the predicted half lives for 4^He and 14^C emission from normal Ac nuclei are favourable for measurement, we presume that alpha and 14^C cluster emission from hyper Ac nuclei can be detected in laboratory in a cascade (two-step) process.

  8. Probable alpha and {sup 14}C cluster emission from hyper Ac nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Santhosh, K.P. [Kannur University, Swami Anandatheertha Campus, School of Pure and Applied Physics, Payyanur (India)

    2013-10-15

    A systematic study on the probability for the emission of {sup 4}He and {sup 14}C cluster from hyper {sub {Lambda}}{sup 207-234}Ac and non-strange normal {sup 207-234}Ac nuclei are performed for the first time using our fission model, the Coulomb and proximity potential model (CPPM). The predicted half lives show that hyper {sub {Lambda}}{sup 207-234}Ac nuclei are unstable against {sup 4}He emission and {sup 14}C emission from hyper {sub {Lambda}}{sup 217-228}Ac are favorable for measurement. Our study also show that hyper {sub {Lambda}}{sup 207-234}Ac are stable against hyper {sub {Lambda}}{sup 4}He and {sub {Lambda}}{sup 14}C emission. The role of neutron shell closure (N = 126) in hyper {sub {Lambda}}{sup 214}Fr daughter and role of proton/neutron shell closure (Z {approx} 82, N = 126) in hyper {sub {Lambda}}{sup 210}Bi daughter are also revealed. As hyper-nuclei decays to normal nuclei by mesonic/non-mesonic decay and since most of the predicted half lives for {sup 4}He and {sup 14}C emission from normal Ac nuclei are favourable for measurement, we presume that alpha and {sup 14}C cluster emission from hyper Ac nuclei can be detected in laboratory in a cascade (two-step) process. (orig.)

  9. Paraboloid Shell As Footing

    OpenAIRE

    Al Ansari, Mohammed S.

    1999-01-01

    A simplified method for the design of paraboloid shell footing base on the displacement of the shell's crown where the column axial load is transferred to the footing has been developed. A case study was presented to demonstrate the use of the proposed method and to illustrate its capabilities. The results of the proposed method confirm the ability of the shell model in determining accurate and practical results for the design of paraboloid shell footing. Base on the analytical results of thi...

  10. Structure and symmetries of odd-odd triaxial nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Palit, R. [Tata Institute of Fundamental Research, Department of Nuclear and Atomic Physics, Colaba, Mumbai (India); Bhat, G.H. [University of Kashmir, Department of Physics, Srinagar (India); Govt. Degree College Kulgam, Department of Physics, Kulgam (India); Sheikh, J.A. [University of Kashmir, Department of Physics, Srinagar (India); Cluster University of Srinagar, Srinagar, Jammu and Kashmir (India)

    2017-05-15

    Rotational spectra of odd-odd Rh and Ag isotopes are investigated with the primary motivation to search for the spontaneous chiral symmetry breaking phenomenon in these nuclei. The experimental results obtained on the degenerate dipole bands of some of these isotopes using a large array of gamma detectors are discussed and studied using the triaxial projected shell (TPSM) approach. It is shown that, first of all, to reproduce the odd-even staggering of the known yrast bands of these nuclei, large triaxial deformation is needed. This large triaxial deformation also gives rise to doublet band structures in many of these studied nuclei. The observed doublet bands in these isotopes are shown to be reproduced reasonably well by the TPSM calculations. Further, the TPSM calculations for neutron-rich nuclei indicate that the ideal manifestation of the chirality can be realised in {sup 106}Rh and {sup 112}Ag, where the doublet bands have similar electromagnetic properties along with small differences in excitation energies. (orig.)

  11. Quantum phase transitions and collective enhancement of level density in odd–A and odd–odd nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Karampagia, S., E-mail: karampag@nscl.msu.edu [National Superconducting Cyclotron Laboratory, Michigan State University, East Lansing, MI 48824-1321 (United States); Renzaglia, A. [Department of Physics and Astronomy, Michigan State University, East Lansing, MI 48824-1321 (United States); Zelevinsky, V. [National Superconducting Cyclotron Laboratory, Michigan State University, East Lansing, MI 48824-1321 (United States); Department of Physics and Astronomy, Michigan State University, East Lansing, MI 48824-1321 (United States)

    2017-06-15

    The nuclear shell model assumes an effective mean-field plus interaction Hamiltonian in a specific configuration space. We want to understand how various interaction matrix elements affect the observables, the collectivity in nuclei and the nuclear level density for odd–A and odd–odd nuclei. Using the sd and pf shells, we vary specific groups of matrix elements and study the evolution of energy levels, transition rates and the level density. In all cases studied, a transition between a “normal” and a collective phase is induced, accompanied by an enhancement of the level density in the collective phase. In distinction to neighboring even–even nuclei, the enhancement of the level density is observed already at the transition point. The collective phase is reached when the single-particle transfer matrix elements are dominant in the shell model Hamiltonian, providing a sign of their fundamental role.

  12. Neutrino absorption by hot nuclei in supernova environments

    CERN Document Server

    Dzhioev, Alan A; Wambach, J

    2015-01-01

    Using the thermal quasiparticle random phase approximation, we study the process of neutrino and antineutrino capture on hot nuclei in supernova environments. For the sample nuclei $^{56}$Fe and $^{82}$Ge we perform a detailed analysis of thermal effects on the strength distribution of allowed Gamow-Teller transitions which dominate low-energy charged-current neutrino reactions. The finite temperature cross sections are calculated taking into account the contributions of both allowed and forbidden transitions. The enhancement of the low-energy cross sections is explained by considering thermal effects on the GT$_\\pm$ strength. For $^{56}$Fe we compare the calculated finite-temperature cross sections with those obtained from large-scale shell-model calculations.

  13. Neutrino absorption by hot nuclei in supernova environments

    Science.gov (United States)

    Dzhioev, Alan A.; Vdovin, A. I.; Wambach, J.

    2015-10-01

    Using the thermal quasiparticle random-phase approximation, we study the process of neutrino and antineutrino capture on hot nuclei in supernova environments. For the sample nuclei 56Fe and 82Ge we perform a detailed analysis of thermal effects on the strength distribution of allowed Gamow-Teller (GT) transitions which dominate low-energy charged-current neutrino reactions. The finite-temperature cross sections are calculated taking into account the contributions of both allowed and forbidden transitions. The enhancement of the low-energy cross sections is explained by considering thermal effects on the GT± strength. For 56Fe we compare the calculated finite-temperature cross sections with those obtained from large-scale shell-model calculations.

  14. Probable Heavy Particle Decays from 306-339128 Superheavy Nuclei

    Science.gov (United States)

    Santhosh, K. P.; Sukumaran, Indu

    2016-12-01

    The heavy particle decays that are probable from the isotopes of Z = 128 superheavy nuclei within the range A = 306-339 have been analyzed within the Coulomb and proximity potential model (CPPM). The study includes the evaluation of heavy particle decay half-lives of 24 clusters, including both odd and even clusters that are supposed to be emitted from the Z = 128 superheavy nuclei. The predicted values in comparison with the models Universal curve (UNIV), Universal decay law (UDL), and scaling law of Horoi et al. are observed to follow the same trend, and almost all the values lie well within the experimental limit ( T 1/2 Geiger-Nuttall plots of log10( T 1/2) vs. Q -1/2 confirming the presence of shell closure effect and the plot of universal curve of log10( T 1 /2) vs.-lnP revealed the reliability of the model CPPM.

  15. Cluster emissions with ? daughter from neutron-rich nuclei

    Science.gov (United States)

    Kumar, Satish; Batra, J. S.; Gupta, Raj K.

    1996-02-01

    Cluster emissions from neutron-rich 0954-3899/22/2/006/img2, and 0954-3899/22/2/006/img3 nuclei are studied within the preformed cluster model of Malik and Gupta. Q-value estimates of the decays selected on the basis of shell effects in binding energies and their relative preformation probabilities show that these nuclei are stable (Qdecays and all the metastable (Q>0) decays are of non-alpha-like heavy clusters. The most probable decays (minimum half-life times) are the ones with a doubly magic 0954-3899/22/2/006/img6 nucleus as the daughter nucleus, arising due to the WKB penetrability. Compared to the presently measurable alpha-like cluster decays of the corresponding neutron-deficient parents into a 0954-3899/22/2/006/img7 daughter nucleus, these decays are suppressed by many orders of magnitude.

  16. Light nuclei in the vicinity of the dripline and beyond

    Energy Technology Data Exchange (ETDEWEB)

    Chulkov, L.V. [GSI Helmholtzzentrum fuer Schwerionenforschung GmbH, Darmstadt (Germany); Kurchatov Institute, Moscow (Russian Federation); Jonson, B.; Zhukov, M.V. [Chalmers Tekniska Hoegskola, Fundamental Fysik, Goeteborg (Sweden)

    2015-08-15

    After a brief historical overview of the field of physics with radioactive beams, we give an update of the most recent experimental achievements for nuclei at or beyond the nuclear driplines. Long-lived exotic nuclear states are discussed including multi-nucleon radioactivity and exotic isomers. Studies of correlations between decay products in three-body decays and analysis in a Jacobi-coordinate framework are discussed with special emphasis on the difficulty in the interpretations of data obtained in different reactions. We give examples of systematic studies that the vast amount of now existing data allows, such as shell closures, competition between single-particle states in isotopes, isotones and mirror nuclei. The Thomas-Ehrman shift, Garvey-Kelson-type mass relations and IMME analysis of isobaric multiplets with isospin T = 3/2 and 2 are also discussed as well as alternative interpretations in certain cases. (orig.)

  17. A nucleon-pair and boson coexistent description of nuclei

    Science.gov (United States)

    Dai, Lianrong; Pan, Feng; Draayer, J. P.

    2017-07-01

    We study a mixture of s-bosons and like-nucleon pairs with the standard pairing interaction outside an inert core. Competition between the nucleon-pairs and s-bosons is investigated in this scenario. The robustness of the BCS-BEC coexistence and crossover phenomena are examined through an analysis of pf-shell nuclei with realistic single-particle energies, in which two configurations with Pauli blocking of nucleon-pair orbits due to the formation of the s-bosons is taken into account. When the nucleon-pair orbits are considered to be independent of the s-bosons, the BCS-BEC crossover becomes smooth, with the number of the s-bosons noticeably more than that of the nucleon-pairs near the half-shell point, a feature that is demonstrated in the pf-shell for several values of the standard pairing interaction strength. As a further test of the robustness of the BCS-BEC coexistence and crossover phenomena in nuclei, results are given for values of even-even 102-130Sn with 100Sn taken as a core and valence neutron pairs confined within the 1d 5/2, 0g 7/2, 1d 3/2, 2s 1/2, 1h 11/2 orbits in the nucleon-pair orbit and the s-boson independent approximation. The results indicate that the B(E2) values are reproduced well. Supported by National Natural Science Foundation of China (11375080, 11675071), the U.S. National Science Foundation (OCI-0904874 and ACI-1516338), U. S. Department of Energy (DE-SC0005248), the Southeastern Universities Research Association, the China-U. S. Theory Institute for Physics with Exotic Nuclei (CUSTIPEN) (DE-SC0009971), and the LSU-LNNU joint research program (9961) is acknowledged

  18. New Vistas of the Structure of Neutron-Rich Nuclei - Single Particle States and g-FACTORS

    Science.gov (United States)

    Ramayya, A. V.; Hamilton, J. H.; Luo, Y. X.; Zhu, S. J.; Hwang, J. K.; Rasmussen, J. O.; Ter-Akopian, G. M.; Daniel, A. V.; Brewer, N.; Oganessian, Y.

    2012-01-01

    Prompt γ-γ-γ coincidence studies of neutron-rich nuclei populated in the spontaneous fission of 252Cf led to the discoveries of many important processes like neutron-less binary and ternary fragmentation in spontaneous fission, binary and ternary hot fission modes, hyper-deformation, cluster radioactivity and quasi-molecular states in ternary fission. The high statistics data, 5.7 × 1011 triples and higher folds, opened up discoveries of new band structures and significant extensions of previously known bands. These data were used to measure the angular correlations of cascades of γ-rays from the excited states of neutron-rich fission fragments stopped in an unmagnetized iron foil. By using this γ-γ angular correlation technique, the single particle configurations of the known rotational bands were assigned and confirmed in the present work. In other words, the multipole mixing ratios of ΔI=1 transitions in the rotational bands were measured. These experimental mixing ratios are compred with the theoretical ones of particle and axial-rotor model. The configuration of the ground states in 109,111Ru were, for the first time, assigned. And magnetic g-factors of excited states in even-even neutron-rich nuclei were meaured, too. Two sets of ΔI=1 alternating parity doublets with opposite parities were observed in Ba and Ce isotopes. The B(E1)/B(E2) branching ratios and D0 values may indicate that the octupole correlations are strong in Ba and Ce isotopes because of the Z=56 and N=88 octupole shell gaps. High-spin, even-parity bands in neutron-rich 108,110,112Ru nuclei indicate two-phonon quasi-gamma bands in 110,112Ru.

  19. Pseudospin Dynamical Symetry in Nuclei

    CERN Document Server

    Ginocchio, Joseph N

    2014-01-01

    Pseudospin symmetry has been useful in understanding atomic nuclei. We review the arguments that this symmetry is a relativistic symmetry. The condition for this symmetry is that the sum of the vector and scalar potentials in the Dirac Hamiltonian is a constant. We give the generators of pseudospin symmetry. We review some of the predictions that follow from this insight into the relativistic origins of pseudospin symmetry. Since in nuclei the sum of the scalar and vector potentials is not zero but is small, we discuss preliminary investigations into the conditions on the potentials to produce partial dynamic pseudospin symmetry. Finally we show that approximate pseudospin symmetry in nuclei predicts approximate spin symmetry in anti-nucleon scattering from nuclei.

  20. Physics with loosely bound nuclei

    Indian Academy of Sciences (India)

    Chhanda Samanta

    2001-08-01

    The essential aspect of contemporary physics is to understand properties of nucleonic matter that constitutes the world around us. Over the years research in nuclear physics has provided strong guidance in understanding the basic principles of nuclear interactions. But, the scenario of nuclear physics changed drastically as the new generation of accelerators started providing more and more rare isotopes, which are away from the line of stability. These weakly bound nuclei are found to exhibit new forms of nuclear matter and unprecedented exotic behaviour. The low breakup thresholds of these rare nuclei are posing new challenges to both theory and experiments. Fortunately, nature has provided a few loosely bound stable nuclei that have been studied thoroughly for decades. Attempts are being made to find a consistent picture for the unstable nuclei starting from their stable counterparts. Some significant differences in the structure and reaction mechanisms are found.

  1. Investigation of exotic modes of spinning nuclei near 90Zr

    Indian Academy of Sciences (India)

    R Palit; S Saha

    2014-04-01

    Recently, a digital data acquisition system with 96 channels has been set up for the Indian National Gamma Array (INGA) consisting of 24 Compton-suppressed clover detectors. The digital system provides higher throughput, better energy resolution and better stability for the multidetector Compton-suppressed clover array compared to the previous conventional system with analog shaping. A number of nuclear spectroscopic experiments have been carried out using the array. Selected results from this array will be presented which highlight different excitations of nuclei near-shell gaps.

  2. Charge symmetry breaking in mirror nuclei from quarks

    CERN Document Server

    Tsushima, K; Thomas, A W

    1999-01-01

    The binding energy differences of the valence proton and neutron of the mirror nuclei, $^{15}$O -- $^{15}$N, $^{17}$F -- $^{17}$O, $^{39}$Ca -- $^{39}$K and $^{41}$Sc -- $^{41}$Ca, are calculated using the quark-meson coupling (QMC) model. The calculation involves nuclear structure and shell effects explicitly. It is shown that binding energy differences of a few hundred keV arise from the strong interaction, even after subtracting all electromagnetic corrections. The origin of these differences may be ascribed to the charge symmetry breaking effects set in the strong interaction through the u and d current quark mass difference.

  3. Numerical Simulation of Effect of Disc Plate's Openings on Shell Side Properties of Coiled Heat Exchanger with Convergent-Divergent Tubes%圆盘板开孔对缩放管盘环式换热器壳程性能影响的数值研究

    Institute of Scientific and Technical Information of China (English)

    吴秋华

    2013-01-01

    利用CFD技术对圆盘板上开不同直径孔的缩放管盘环式换热器壳程进行了数值模拟.结果表明,田盘板开孔能在一定程度上改善圆盘板后侧流体的流动状况,且开孔后圆盘与圆环折流板之间的流体压力分布较均匀;开孔直径越大,挟热器的壳程传热系数和压降均越小,综合性能越好;开孔直径不宜过小,适当地开孔才能有效地提高换热器的综合性能.%Making use of CFD,the shell side properties of coiled heat exchanger with convergent — divergent tubes were simulated.The results show that,the disc plate' s opening can improve fluid' s flow condition at disc plate' s rear side and can bring a well-distributed fluid pressure between disc and baffle plate ; and the openings'larger diameter can bring smaller shell side heat transfer coefficient and pressure drop.The opening's proper diameter can benefit the improvement of comprehensive properties of heat exchangers.

  4. Systematic study of survival probability of excited superheavy nuclei

    Institute of Scientific and Technical Information of China (English)

    2011-01-01

    The stability of excited superheavy nuclei (SHN) with 100 Z 134 against neutron emission and fission is investigated by using a statistical model. In particular, a systematic study of the survival probability against fission in the 1n-channel of these SHN is made. The present calculations consistently take the neutron separation energies and shell correction energies from the calculated results of the finite range droplet model which predicts an island of stability of SHN around Z = 115 and N = 179. It turns out that this island of stability persists for excited SHN in the sense that the calculated survival probabilities in the 1n-channel of excited SHN at the optimal excitation energy are maximized around Z = 115 and N = 179. This indicates that the survival probability in the 1n-channel is mainly determined by the nuclear shell effects.

  5. The structure of 100Sn and neighbouring nuclei

    Science.gov (United States)

    Faestermann, T.; Górska, M.; Grawe, H.

    2013-03-01

    The nuclear structure in the 100Sn region is reviewed. State-of-the-art experimental techniques involving stable and radioactive beam facilities have enabled access to exotic nuclei in its next neighbourhood. The analysis of experimental data has established the shell structure and its evolution towards N=Z=50, seniority conservation and proton-neutron interaction in the g9/2 orbit, the super-allowed Gamow-Teller decay of 100Sn, masses and half lives along the rp-path, and super-allowed α decay beyond 100Sn. The status of theoretical approaches in shell model and mean-field investigations is described and their predictive power assessed. Structure features of 100Sn and its doubly-magic neighbours 56Ni at N=Z, 132Sn and 78Ni at N≫Z are compared. An outlook is given on future developments of experimental and theoretical methods.

  6. Nuclear spectroscopy in nuclei with Z ≥ 110

    Energy Technology Data Exchange (ETDEWEB)

    Ackermann, D., E-mail: D.Ackermann@gsi.de

    2015-12-15

    The nuclear structure of species at the extreme of highest atomic numbers Z and nuclear masses A promises to reveal intriguing new features of this exotic hadronic matter. Their stability itself they owe to quantum-mechanic effects only. They form metastable states which, governed by the subtle interplay of α decay and spontaneous fission versus quantum-mechanic stabilization via shell effects, are in some cases more robust against disintegration than their ground states. Following the isotopic and isotonic trends of single particle levels, as well as collective features like deformation, may reveal the path towards the gap in the level densities, expected for the next closed proton and neutron shells at the so-called “island of stability” of spherical superheavy nuclei. Their atomic configuration offers via X-ray spectroscopy a tool to identify the atomic number of heavy species, where other more traditional methods like evaporation residue (ER)–α correlation are not applicable.

  7. Ground-state properties of neutron magic nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Saxena, G., E-mail: gauravphy@gmail.com [Govt. Women Engineering College, Department of Physics (India); Kaushik, M. [Shankara Institute of Technology, Department of Physics (India)

    2017-03-15

    A systematic study of the ground-state properties of the entire chains of even–even neutron magic nuclei represented by isotones of traditional neutron magic numbers N = 8, 20, 40, 50, 82, and 126 has been carried out using relativistic mean-field plus Bardeen–Cooper–Schrieffer approach. Our present investigation includes deformation, binding energy, two-proton separation energy, single-particle energy, rms radii along with proton and neutron density profiles, etc. Several of these results are compared with the results calculated using nonrelativistic approach (Skyrme–Hartree–Fock method) along with available experimental data and indeed they are found with excellent agreement. In addition, the possible locations of the proton and neutron drip-lines, the (Z, N) values for the new shell closures, disappearance of traditional shell closures as suggested by the detailed analyzes of results are also discussed in detail.

  8. Shape coexistence: the shell model view

    Science.gov (United States)

    Poves, A.

    2016-02-01

    We shall discuss the meaning of the ‘nuclear shape’ in the laboratory frame proper to the spherical shell model. A brief historical promenade will bring us from Elliott’s SU3 breakthrough to today’s large scale shell model calculations. A section is devoted to the algebraic model which extends drastically the field of applicability of Elliot’s SU3, providing a precious heuristic guidance for the exploration of collectivity in the nuclear chart. Shape coexistence and shape mixing will be shown to occur as the result of the competition between the main actors in the nuclear dynamics; the spherical mean field, and the pairing and quadrupole-quadrupole interactions. These ideas will be illustrated with examples in magic nuclei (40Ca and 68Ni); neutron rich semi-magic (32Mg, and 64Cr); and in proton rich N = Z (72Kr).

  9. Comparison of β-decay and Charge-exchange Reactions in Mirror T=2 Nuclei and Isospin Mixing

    Institute of Scientific and Technical Information of China (English)

    B Rubio; A Poves; S E A Orrigo; A Algora; B Blank; Y Fujita; H Fujita; E Ganioglu; W Gelletly; A Montaner-Piza

    2016-01-01

    We have carried outβdecay studies of proton rich nuclei in the fp shell at different laboratories. Here we present our recent results on the β decay of Tz=−2 nuclei performed at GANIL and compare them with the Charge Exchange reactions on their stable, mirror-partner targets, performed at RCNP. In one of the cases, the 56Zn- 56Fe pair, a strong isospin mixing has been observed. The results are well reproduced in the framework of Shell Model calculations.

  10. Spectroscopy of low-lying states in neutron-deficient astatine and francium nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Jakobsson, U., E-mail: ulrjak@kth.se; Cederwall, B. [KTH, The Division of Nuclear Physics, AlbaNova University Center, SE-10691 Stockholm (Sweden); Uusitalo, J.; Auranen, K.; Badran, H.; Cox, D. M.; Grahn, T.; Greenlees, P. T.; Julin, R.; Juutinen, S.; Herzáň, A.; Konki, J.; Leino, M.; Mallaburn, M.; Pakarinen, J.; Papadakis, P.; Partanen, J.; Rahkila, P.; Sandzelius, M.; Sarén, J. [University of Jyvaskyla, Department of Physics, P.O. Box 35, FI-40014 University of Jyvaskyla (Finland); and others

    2015-10-15

    Low-lying states in neutron-deficient astatine and francium nuclei have been studied by means of in-beam and delayed spectroscopy. The 13/2{sup +} state has been observed in francium nuclei with a similar down-sloping trend as in neighbouring astatine and bismuth isotopes, as a function of decreasing neutron number. A systematic trend can also now be seen for the 1/2{sup +} state both in astatine and francium nuclei, where the level energy decreases steeply as a function of neutron number when moving further away from the neutron shell closure. This trend is very similar between astatine nuclei and their francium isotones. Moreover, shape coexistence has been observed between the 13/2{sup +} state and the spherical 9/2{sup −} ground state in {sup 203}Fr and {sup 205}Fr.

  11. No-Core Shell Model for 48-Ca, 48-Sc and 48-Ti

    Energy Technology Data Exchange (ETDEWEB)

    Popescu, S; Stoica, S; Vary, J P; Navratil, P

    2004-10-26

    The authors report the first no-core shell model results for {sup 48}Ca, {sup 48}Sc and {sup 48}Ti with derived and modified two-body Hamiltonians. We use an oscillator basis with a limited {bar h}{Omega} range around 40/A{sup 1/3} = 11 MeV and a limited model space up to 1 {bar h}{Omega}. No single-particle energies are used. They find that the charge dependence of the bulk binding energy of eight A = 48 nuclei is reasonably described with an effective Hamiltonian derived from the CD-Bonn interaction while there is an overall underbinding by about 0.4 MeV/nucleon. However, resulting spectra exhibit deficiencies that are anticipated due to: (1) basis space limitations and/or the absence of effective many-body interactions; and, (2) the absence of genuine three-nucleon interactions. They introduce phenomenological modifications to obtain fits to total binding and low-lying spectra. The resulting no-core shell model opens a path for applications to experiments such as the double-beta ({beta}{beta}) decay process.

  12. Shell structure and few-nucleon removal in intranuclear cascade

    CERN Document Server

    Mancusi, Davide; Carbonell, Jaume; Cugnon, Joseph; David, Jean-Christophe; Leray, Sylvie

    2014-01-01

    It is well known that intranuclear-cascade models generally overestimate the cross sections for one-proton removal from heavy, stable nuclei by a high-energy proton beam, but they yield reasonable predictions for one-neutron removal from the same nuclei and for one-nucleon removal from light targets. We use simple shell-model calculations to investigate the reasons of this deficiency. We find that a correct description of the neutron skin and of the energy density in the nuclear surface is crucial for the aforementioned observables. Neither ingredient is sufficient if taken separately.

  13. Signatures of shell evolution in alpha decay across the N = 126 shell closure

    Science.gov (United States)

    Rui-Wang; Wang, Rui-Yao; Qian, Yi-Bin; Ren, Zhong-Zhou

    2017-06-01

    Within the alpha-cluster model, we particularly investigate the alpha decay of exotic nuclei in the vicinity of the N = 126 neutron shell plus the Z = 82 proton shell. The systematics of alpha-preformation probability (P α ), as an indicator of the shell effect, is deduced from the ratio of the experimental decay width to the calculated one. Through the comparative analysis of the P α trend in the N = 124-130 isotonic chain, the N = 126 and Z = 82 shell closures are believed to strongly affect the formation of the alpha particle before its penetration. Additionally, the P α variety in Po and Rn isotopes is presented as another proof for such an influence. More importantly, it may be concluded that the expected neutron (or proton) shell effect gradually fades away along with the increasing valence proton (or neutron) number. The odd-even staggering presented in the P α value is also discussed. Supported by National Natural Science Foundation of China (11375086, 11535004, 11605089, 11120101005), Natural Science Youth Fund of Jiangsu Province (BK20150762), Fundamental Research Funds for the Central Universities (30916011339), 973 National Major State Basic Research and Development Program of China (2013CB834400), and a Project Funded by the Priority Academic Programme Development of JiangSu Higher Education Institutions (PAPD)

  14. Unstable nuclei in dissociation of light stable and radioactive nuclei in nuclear track emulsion

    CERN Document Server

    Artemenkov, D A; Zarubin, P I

    2016-01-01

    A role of the unstable nuclei ${}^{6}$Be, ${}^{8}$Be and ${}^{9}$B in the dissociation of relativistic nuclei ${}^{7,9}$Be, ${}^{10}$B and ${}^{10,11}$C is under study on the basis of nuclear track emulsion exposed to secondary beams of the JINR Nuclotron. Contribution of the configuration ${}^{6}$Be + $\\mit{n}$ to the ${}^{7}$Be nucleus structure is 8 $\\pm$ 1% which is near the value for the configuration ${}^{6}$Li + $\\mit{p}$. Distributions over the opening angle of $\\alpha$-particle pairs indicate to a simultaneous presence of virtual ${}^{8}$Be$_{g.s.}$ and ${}^{8}$Be$_{2^+}$ states in the ground states of the ${}^{9}$Be and ${}^{10}$C nuclei. The core ${}^{9}$B is manifested in the {${}^{10}$C} nucleus with a probability of 30 $\\pm$ 4%. Selection of the ${}^{10}$C "white" stars accompanied by ${}^{8}$Be$_{g.s.}$ (${}^{9}$B) leads to appearance in the excitation energy distribution of 2$\\alpha$2$\\mit{p}$ "quartets" of the distinct peak with a maximum at 4.1 $\\pm$ 0.3 MeV. ${}^{8}$Be$_{g.s.}$ decays are p...

  15. Ab Initio No-Core Shell Model Calculations Using Realistic Two- and Three-Body Interactions

    Energy Technology Data Exchange (ETDEWEB)

    Navratil, P; Ormand, W E; Forssen, C; Caurier, E

    2004-11-30

    There has been significant progress in the ab initio approaches to the structure of light nuclei. One such method is the ab initio no-core shell model (NCSM). Starting from realistic two- and three-nucleon interactions this method can predict low-lying levels in p-shell nuclei. In this contribution, we present a brief overview of the NCSM with examples of recent applications. We highlight our study of the parity inversion in {sup 11}Be, for which calculations were performed in basis spaces up to 9{Dirac_h}{Omega} (dimensions reaching 7 x 10{sup 8}). We also present our latest results for the p-shell nuclei using the Tucson-Melbourne TM three-nucleon interaction with several proposed parameter sets.

  16. Testing refined shell-model interactions in the sd shell: Coulomb excitation of Na26

    CERN Document Server

    Siebeck, B; Blazhev, A; Reiter, P; Altenkirch, R; Bauer, C; Butler, P A; De Witte, H; Elseviers, J; Gaffney, L P; Hess, H; Huyse, M; Kröll, T; Lutter, R; Pakarinen, J; Pietralla, N; Radeck, F; Scheck, M; Schneiders, D; Sotty, C; Van Duppen, P; Vermeulen, M; Voulot, D; Warr, N; Wenander, F

    2015-01-01

    Background: Shell-model calculations crucially depend on the residual interaction used to approximate the nucleon-nucleon interaction. Recent improvements to the empirical universal sd interaction (USD) describing nuclei within the sd shell yielded two new interactions—USDA and USDB—causing changes in the theoretical description of these nuclei. Purpose: Transition matrix elements between excited states provide an excellent probe to examine the underlying shell structure. These observables provide a stringent test for the newly derived interactions. The nucleus Na26 with 7 valence neutrons and 3 valence protons outside the doubly-magic 16O core is used as a test case. Method: A radioactive beam experiment with Na26 (T1/2=1,07s) was performed at the REX-ISOLDE facility (CERN) using Coulomb excitation at safe energies below the Coulomb barrier. Scattered particles were detected with an annular Si detector in coincidence with γ rays observed by the segmented MINIBALL array. Coulomb excitation cross sections...

  17. Delayed neutron emission near the shell-closures

    Directory of Open Access Journals (Sweden)

    Borzov Ivan

    2016-01-01

    Full Text Available The self-consistent Density Functional + Continuum QRPA approach (DF+CQRPA provides a good description of the recent experimental beta-decay half-lives and delayed neutron emission branchings for the nuclei approaching to (and beyond the neutron closed shells N = 28; 50; 82. Predictions of beta-decay properties are more reliable than the ones of standard global approaches traditionally used for the r-process modelling. An impact of the quasi-particle phonon coupling on the delayed multi-neutron emission rates P2n, P3n,… near the closed shells is also discussed.

  18. Photodissociation of neutron deficient nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Sonnabend, K.; Babilon, M.; Hasper, J.; Mueller, S.; Zarza, M.; Zilges, A. [TU Darmstadt, Institut fuer Kernphysik, Darmstadt (Germany)

    2006-03-15

    The knowledge of the cross sections for photodissociation reactions like e.g. ({gamma}, n) of neutron deficient nuclei is of crucial interest for network calculations predicting the abundances of the so-called p nuclei. However, only single cross sections have been measured up to now, i.e., one has to rely nearly fully on theoretical predictions. While the cross sections of stable isotopes are accessible by experiments using real photons, the bulk of the involved reactions starts from unstable nuclei. Coulomb dissociation (CD) experiments in inverse kinematics might be a key to expand the experimental database for p-process network calculations. The approach to test the accuracy of the CD method is explained. (orig.)

  19. A relativistic symmetry in nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Ginocchio, J N [MS B283, Theoretical Division, Los Alamos National Laboratory Los Alamos, New Mexico 87545 (Mexico)

    2007-11-15

    We review some of the empirical and theoretical evidence supporting pseudospin symmetry in nuclei as a relativistic symmetry. We review the case that the eigenfunctions of realistic relativistic nuclear mean fields approximately conserve pseudospin symmetry in nuclei. We discuss the implications of pseudospin symmetry for magnetic dipole transitions and Gamow-Teller transitions between states in pseudospin doublets. We explore a more fundamental rationale for pseudospin symmetry in terms of quantum chromodynamics (QCD), the basic theory of the strong interactions. We show that pseudospin symmetry in nuclei implies spin symmetry for an anti-nucleon in a nuclear environment. We also discuss the future and what role pseudospin symmetry may be expected to play in an effective field theory of nucleons.

  20. Photoproduction of mesons off nuclei

    CERN Document Server

    Krusche, B

    2011-01-01

    Recent results for the photoproduction of mesons off nuclei are reviewed. These experiments have been performed for two major lines of research related to the properties of the strong interaction. The investigation of nucleon resonances requires light nuclei as targets for the extraction of the isospin composition of the electromagnetic excitations. This is done with quasi-free meson photoproduction off the bound neutron and supplemented with the measurement of coherent photoproduction reactions, serving as spin and/or isospin filters. Furthermore, photoproduction from light and heavy nuclei is a very efficient tool for the study of the interactions of mesons with nuclear matter and the in-medium properties of hadrons. Experiments are currently rapidly developing due to the combination of high quality tagged (and polarized) photon beams with state-of-the-art 4pi detectors and polarized targets.

  1. Production Uncertainties of p-Nuclei in the γ-Process in Massive Stars Using a Monte Carlo Approach

    Science.gov (United States)

    Rauscher, T.; Nishimura, N.; Hirschi, R.; Cescutti, G.; Murphy, A. St. J.; Heger, A.

    Proton-rich nuclei, the so-called p-nuclei, are made in photodisintegration processes in outer shells of massive stars in the course of the final supernova explosion. Nuclear uncertainties in the production of these nuclei have been quantified in a Monte Carlo procedure. Bespoke temperature-dependent uncertainties were assigned to different types of reactions involving nuclei from Fe to Bi and all rates were varied randomly within the uncertainties. The resulting total production uncertainties of the p-nuclei are below a factor of two, with few exceptions. Key reactions dominating the final uncertainties have been identified in an automated procedure using correlations between rate and abundance uncertainties. Our results are compared to those of a previous study manually varying reaction rates.

  2. Production Uncertainties of p-Nuclei in the $\\gamma$-Process in Massive Stars Using a Monte Carlo Approach

    CERN Document Server

    Rauscher, T; Hirschi, R; Cescutti, G; Murphy, A St J; Heger, A

    2016-01-01

    Proton-rich nuclei, the so-called p-nuclei, are made in photodisintegration processes in outer shells of massive stars in the course of the final supernova explosion. Nuclear uncertainties in the production of these nuclei have been quantified in a Monte Carlo procedure. Bespoke temperature-dependent uncertainties were assigned to different types of reactions involving nuclei from Fe to Bi and all rates were varied randomly within the uncertainties. The resulting total production uncertainties of the p-nuclei are below a factor of two, with few exceptions. Key reactions dominating the final uncertainties have been identified in an automated procedure using correlations between rate and abundance uncertainties. Our results are compared to those of a previous study manually varying reaction rates.

  3. Tom W. Bonner Prize in Nuclear Physics Talk: Symmetries and Simple Patterns in Nuclei

    Science.gov (United States)

    Casten, Richard

    2011-04-01

    Nuclei are complex many-body objects that display remarkably simple patterns and regularities, both for a given nucleus and across regions of nuclei. The juxtaposition of these two facets of nuclear structure is reflected in two general, and complementary, approaches to their description - a microscopic (femtoscopic, of course) perspective in terms of the motions of the individual nucleons and their interactions, and a macroscopic view of the nucleus as a whole, in terms of its shapes, symmetries, and collective behavior. The first part of this talk will discuss the simple patterns nuclei exhibit and interpret them in terms of symmetries, such as those of the Interacting Boson Approximation (IBA) model, elementary collective modes, changes in shell structure, and quantum phase transitions in the equilibrium structure. It is also possible to approach structural evolution in nuclei with an extremely simple, more microscopic, perspective focusing on the competition of the most important residual interactions, pairing and the valence proton-neutron (p - n) interaction. While this is not a substitute for a comprehensive theoretical treatment, which remains a challenge and goal of nuclear theory, such an analysis leads to simple approaches, such as the NpNn scheme and the P-factor, that correlate large amounts of nuclear data, can guide estimates of unknown nuclei, and which are highly sensitive indicators of changes in shell structure and of nuclei that exhibit behavior deviating from normal tends. Finally, empirical means of extracting information on the critical valence p - n interaction will be discussed and the systematic behavior of these interaction strengths will be linked to shell structure on the one hand, and the onset and development of collectivity on the other. Work supported by the US DOE under Grant No. DE-FG02-91ER-40609.

  4. Spiral Shell Collection

    Institute of Scientific and Technical Information of China (English)

    1995-01-01

    In 1988 Zheng Haigen, a seaman with the Towboat Company of the Shanghai Salvage Bureau, began collecting spiral shells. Today he has more than 600 in his collection. The most valuable are the rare parrot shell and a shell whose spirals wind counter-clockwise. In 1991 a miniature conch with a diameter of 0.31 millimeters that he found buried in tons of sand made the Guinness Book of World Records.

  5. Off-Shell Tachyons

    OpenAIRE

    Tang, Yi-Lei

    2015-01-01

    The idea that the new particles invented in some models beyond the standard model can appear only inside the loops is attractive. In this paper, we fill these loops with off-shell tachyons, leading to a solution of the zero results of the loop diagrams involving the off-shell non-tachyonic particles. We also calculate the Passarino-Veltman $A_0^o$ and $B_0^o$ of the off-shell tachyons.

  6. Long-range correlations and the momentum distribution in nuclei

    CERN Document Server

    Amir-Azimi-Nili, K; Skouras, L D; Polls, A

    1996-01-01

    The influence of correlations on the momentum distribution of nucleons in nuclei is evaluated starting from a realistic nucleon-nucleon interaction. The calculations are performed directly for the finite nucleus \\,^{16}O making use of the Green's function approach. The emphasis is focused on the correlations induced by the excitation modes at low energies described within a model-space of shell-model configurations including states up to the sdg shell. Our analysis demonstrates that these long-range correlations do not produce any significant enhancement of the momentum distribution at high missing momenta and low missing energies. This is in agreement with high resolution (e,e'p) experiments for this nucleus. We also try to simulate the corresponding effects in large nuclei by quenching the energy-spacing between single-particle orbits. This yields a sizable enhancement of the spectral function at large momenta and small energy. Such behavior could explain the deviation of the momentum distribution from the ...

  7. Quartetting in odd-odd self-conjugate nuclei

    CERN Document Server

    Sambataro, M

    2016-01-01

    We provide a description of odd-odd self-conjugate nuclei in the sd shell in a formalism of collective quartets and pairs. Quartets are four-body structures carrying isospin T=0 while pairs can have either T=0 or T=1. Both quartets and pairs are labeled by the angular momentum J and they are chosen so as to describe the lowest states of 20Ne (quartets) and the lowest T=0 and T=1 states of 18F (pairs). We carry out configuration interaction calculations in spaces built by one quartet and one pair for 22Na and by two quartets and one pair for 26Al. The spectra that are generated are in good agreement with the shell model and experimental ones. These calculations confirm the relevance of quartetting in the structure of N=Z nuclei that had already emerged in previous studies of the even-even systems and highlight the role of J>0 quartets in the composition of the odd-odd spectra.

  8. Octupole shapes in heavy nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Ahmad, I.

    1994-08-01

    Theoretical calculations and measurements show the presence of strong octupole correlations in thecyround states and low-lying states of odd-mass and odd-odd nuclei in the RaPa region. Evidence for octupole correlations is provided by the observation of parity doublets and reductions in M1 matrix elements, decoupling parameters, and Coriolis matrix elements Involving high-j states. Enhancement of E1 transition rates has also been observed for some of the octupole deformed nuclei. The most convincing argument for octupole deformation is provided by the similarities of the reduced alpha decay rates to the two members of parity doublets.

  9. International Symposium on Exotic Nuclei

    CERN Document Server

    Sobolev, Yu G; EXON-2014

    2015-01-01

    The production and the properties of nuclei in extreme conditions, such as high isospin, temperature, angular momenta, large deformations etc., have become the subject of detailed investigations in all scientific centers. The main topics discussed at the Symposium were: Synthesis and Properties of Exotic Nuclei; Superheavy Elements; Rare Processes, Nuclear Reactions, Fission and Decays; Experimental Facilities and Scientific Projects. This book provides a comprehensive overview of the newest results of the investigations in the main scientific centers such as GSI (Darmstadt, Germany), GANIL (Caen, France), RIKEN (Wako-shi, Japan), MSU (Michigan, USA), and JINR (Dubna, Russia).

  10. PDFs from nucleons to nuclei

    CERN Document Server

    Accardi, Alberto

    2016-01-01

    I review recent progress in the extraction of unpolarized parton distributions in the proton and in nuclei from a unified point of view that highlights how the interplay between high energy particle physics and lower energy nuclear physics can be of mutual benefit to either field. Areas of overlap range from the search for physics beyond the standard model at the LHC, to the study of the non perturbative structure of nucleons and the emergence of nuclei from quark and gluon degrees of freedom, to the interaction of colored probes in a cold nuclear medium.

  11. Dynamics and Control of Adaptive Shells with Curvature Transformations

    Directory of Open Access Journals (Sweden)

    H.S. Tzou

    1995-01-01

    Full Text Available Adaptive structures with controllable geometries and shapes are rather useful in many engineering applications, such as adaptive wings, variable focus mirrors, adaptive machines, micro-electromechanical systems, etc. Dynamics and feedback control effectiveness of adaptive shells whose curvatures are actively controlled and continuously changed are evaluated. An adaptive piezoelectric laminated cylindrical shell composite with continuous curvature changes is studied, and its natural frequencies and controlled damping ratios are evaluated. The curvature change of the adaptive shell starts from an open shallow shell (30° and ends with a deep cylindrical shell (360°. Dynamic characteristics and control effectiveness (via the proportional velocity feedback of this series of shells are investigated and compared at every 30° curvature change. Analytical solutions suggest that the lower modes are sensitive to curvature changes and the higher modes are relatively insensitive.

  12. Shell-like structures

    CERN Document Server

    Altenbach, Holm

    2011-01-01

    In this volume, scientists and researchers from industry discuss the new trends in simulation and computing shell-like structures. The focus is put on the following problems: new theories (based on two-dimensional field equations but describing non-classical effects), new constitutive equations (for materials like sandwiches, foams, etc. and which can be combined with the two-dimensional shell equations), complex structures (folded, branching and/or self intersecting shell structures, etc.) and shell-like structures on different scales (for example: nano-tubes) or very thin structures (similar

  13. Dynamical effects in fusion with exotic nuclei

    CERN Document Server

    Vo-Phuoc, K; Simpson, E C

    2016-01-01

    [Background] Reactions with stable beams have demonstrated a strong interplay between nuclear structure and fusion. Exotic beam facilities open new perspectives to understand the impact of neutron skin, large isospin, and weak binding energies on fusion. Microscopic theories of fusion are required to guide future experiments. [Purpose] To investigate new effects of exotic structures and dynamics in near-barrier fusion with exotic nuclei. [Method] Microscopic approaches based on the Hartree-Fock (HF) mean-field theory are used for studying fusion barriers in $^{40-54}$Ca+$^{116}$Sn reactions for even isotopes. Bare potential barriers are obtained assuming frozen HF ground-state densities. Dynamical effects on the barrier are accounted for in time-dependent Hartree-Fock (TDHF) calculations of the collisions. Vibrational couplings are studied in the coupled-channel framework and near-barrier nucleon transfer is investigated with TDHF calculations. [Results] The development of a neutron skin in exotic calcium iso...

  14. Theoretical Emission-Line Profiles of Active Galactic Nuclei and the Unified Model. I. The Face-on Torus

    Science.gov (United States)

    Quintilio, R.; Viegas, S. M.

    1997-01-01

    Theoretical emission-line profiles are obtained for active galactic nuclei (AGNs) taking into account the presence of an obscuring torus around the central energy source. For the sake of simplicity, the torus is represented by a cylindrical shell characterized by the inner and outer radius and the opening angle. In this paper we discuss the results with angle of sight equal to 0, i.e., for a face-on torus. Different line profiles are obtained following the torus parameters. The line profiles may show more than one peak and bumps, depending on the torus dimensions. The main parameter determining the number of peaks or bumps is the opening angle. Thus, the observed line shape may be a good indicator of the torus characteristics. As an example, the fit to the observed [O III] λ5007 emission line of NGC 4151 is presented. The model reproduces the FWHM and the asymmetrical bumps observed. Partially supported by the Fundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP) under Grant 92/4335-9.

  15. Transition from the Seniority to the Anharmonic Vibrator Regime in Nuclei

    CERN Document Server

    Bijker, R; Pittel, S

    1996-01-01

    A recent analysis of experimental energy systematics suggests that all collective nuclei fall into one of three classes -- seniority, anharmonic vibrational, or rotational -- with sharp phase transitions between them. We investigate the transition from the seniority to the anharmonic vibrator regime within a shell model framework involving a single large j-orbit. The calculations qualitatively reproduce the observed transitional behavior, both for U(5) like and O(6) like nuclei. They also confirm the preeminent role played by the neutron-proton interaction in producing the phase transition.

  16. Cluster decay analysis and related structure effects of fissionable heavy and superheavy nuclei

    Indian Academy of Sciences (India)

    Manoj K Sharma; Gurvinder Kaur

    2015-09-01

    Collective clusterization approach of dynamical cluster decay model (DCM) has been applied to study the attributes of hot ( ≠ 0) and rotating (ℓ = 0) nuclei lying in heavy and super-heavy mass regimes. We present here an overview of the characteristic fission decay properties such as shell effect, role of entrance channel, quadrupole (2) deformations and impact of hot (equatorial) compact orientation degree of freedom in comparison to cold (polar) elongated configuration. The presence of non-compound nucleus process, i.e., quasifission, is also investigated. Apart from studying the decay of excited state nuclei, the dynamics of heavy particle cluster emission is also addressed using the preformed cluster model (PCM).

  17. Properties of the Alpha Decay Chain Nuclei of 310126, 292120 and 298114

    Institute of Scientific and Technical Information of China (English)

    WANG Ting-Tai; JIANG Wei-Zhou; ZHANG Wei; WANG Kun; ZHU Zhi-Yuan

    2004-01-01

    @@ The properties of the α decay nuclei of 310126, 292120 and 298 114 are investigated in the deformed relativistic meanfield model. The nuclear properties are investigated with the TMA and NL-Z2 parameter sets, and comparedwith Moller's result [At. Data Nucl. Data Tables 59 (1995) 185]. The results show that the α decay energy increases systematically with the increasing proton number. Meanwhile, the a decay energy has a minimum value at the point of shell closure. It is also found that among the three nuclei, 292120 is more possible to be the next doubly magic nucleus.

  18. Shell quenching in Ni78: A hint from the structure of neutron-rich copper isotopes

    Science.gov (United States)

    Sieja, K.; Nowacki, F.

    2010-06-01

    Recent progress in experimental techniques allows us to study very exotic systems like neutron-rich nuclei in the vicinity of Ni78. The spectroscopy of this region can nowadays be studied theoretically in the large scale shell model calculations. In this work, we perform a shell model study of odd copper nuclei with N=40-50, in a large valence space with the Ca48 core, using a realistic interaction derived from the CD-Bonn potential. We present the crucial importance of the proton core excitations for the description of spectra and magnetic moments, which are for the first time correctly reproduced in theoretical calculations. Shell evolution from Ni68 to Ni78 is discussed in detail. A weakening of the Z=28 gap when approaching the N=50 shell closure, suggested by the experimental evidence, is confirmed in the calculations.

  19. Engineered inorganic core/shell nanoparticles

    Energy Technology Data Exchange (ETDEWEB)

    Mélinon, Patrice, E-mail: patrice.melinon@univ-lyon1.fr [Institut Lumière matière Université Claude Bernard Lyon 1 et CNRS et OMNT, Domaine Scientifique de la Doua, Bâtiment Léon Brillouin, 43 Boulevard du 11 Novembre 1918, F 69622 Villeurbanne (France); Begin-Colin, Sylvie [IPCMS et OMNT, 23 rue du Loess BP 43, 67034 STRASBOURG Cedex 2 (France); Duvail, Jean Luc [IMN UMR 6502 et OMNT Campus Sciences : 2 rue de la Houssinire, BP32229, 44322 Nantes Cedex3 (France); Gauffre, Fabienne [SPM et OMNT : Institut des sciences chimiques de Rennes - UMR 6226, 263 Avenue du General Leclerc, CS 74205, 35042 RENNES Cedex (France); Boime, Nathalie Herlin [IRAMIS-NIMBE, Laboratoire Francis Perrin (CEA CNRS URA 2453) et OMNT, Bat 522, CEA Saclay, 91191 Gif sur Yvette Cedex (France); Ledoux, Gilles [Institut Lumière Matière Université Claude Bernard Lyon 1 et CNRS et OMNT, Domaine Scientifique de la Doua, Bâtiment Alfred Kastler 43 Boulevard du 11 Novembre 1918 F 69622 Villeurbanne (France); Plain, Jérôme [Universit de technologie de Troyes LNIO-ICD, CNRS et OMNT 12 rue Marie Curie - CS 42060 - 10004 Troyes cedex (France); Reiss, Peter [CEA Grenoble, INAC-SPrAM, UMR 5819 CEA-CNRS-UJF et OMNT, Grenoble cedex 9 (France); Silly, Fabien [CEA, IRAMIS, SPEC, TITANS, CNRS 2464 et OMNT, F-91191 Gif sur Yvette (France); Warot-Fonrose, Bénédicte [CEMES-CNRS, Université de Toulouse et OMNT, 29 rue Jeanne Marvig F 31055 Toulouse (France)

    2014-10-20

    It has been for a long time recognized that nanoparticles are of great scientific interest as they are effectively a bridge between bulk materials and atomic structures. At first, size effects occurring in single elements have been studied. More recently, progress in chemical and physical synthesis routes permitted the preparation of more complex structures. Such structures take advantages of new adjustable parameters including stoichiometry, chemical ordering, shape and segregation opening new fields with tailored materials for biology, mechanics, optics magnetism, chemistry catalysis, solar cells and microelectronics. Among them, core/shell structures are a particular class of nanoparticles made with an inorganic core and one or several inorganic shell layer(s). In earlier work, the shell was merely used as a protective coating for the core. More recently, it has been shown that it is possible to tune the physical properties in a larger range than that of each material taken separately. The goal of the present review is to discuss the basic properties of the different types of core/shell nanoparticles including a large variety of heterostructures. We restrict ourselves on all inorganic (on inorganic/inorganic) core/shell structures. In the light of recent developments, the applications of inorganic core/shell particles are found in many fields including biology, chemistry, physics and engineering. In addition to a representative overview of the properties, general concepts based on solid state physics are considered for material selection and for identifying criteria linking the core/shell structure and its resulting properties. Chemical and physical routes for the synthesis and specific methods for the study of core/shell nanoparticle are briefly discussed.

  20. Inelastic neutrino scattering off hot nuclei in supernova environments

    Science.gov (United States)

    Dzhioev, Alan A.; Vdovin, A. I.; Wambach, J.; Ponomarev, V. Yu.

    2014-03-01

    We study inelastic neutrino scattering off hot nuclei for temperatures relevant under supernova conditions. The method we use is based on the quasiparticle random phase approximation extended to finite temperatures within the thermo-field dynamics. The method allows a transparent treatment of upward and downward transitions in hot nuclei, avoiding the application of Brink's hypothesis. For the sample nuclei 56Fe and 82Ge we perform a detailed analysis of thermal effects on the strength distributions of allowed Gamow-Teller (GT) transitions which dominate the scattering process at low neutrino energies. For 56Fe and 82Ge the finite temperature cross sections are calculated by taking into account the contribution of allowed and forbidden transitions. The observed enhancement of the cross section at low neutrino energies is explained by considering thermal effects on the GT strength. For 56Fe we compare the calculated cross sections to those obtained earlier from a hybrid approach that combines large-scale shell-model and RPA calculations.

  1. Classically dynamical behaviour of a nucleon in heavy nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Gu Jianzhong [CCAST World Lab., Beijing, BJ (China)]|[Institute of Theoretical Physics, Academia Sinica, P.O. Box 2735, Beijing, 100080 (China); Zhao Enguang; Zong Hongshi [Institute of Theoretical Physics, Academia Sinica, P.O. Box 2735, Beijing, 100080 (China); Zhuo Yizhong [Institute of Theoretical Physics, Academia Sinica, P.O. Box 2735, Beijing, 100080 (China)]|[China Institute of Atomic Energy, P.O. Box 275 18, Beijing, 102413 (China); Wu Xizhen [China Institute of Atomic Energy, P.O. Box 275 18, Beijing, 102413 (China)

    1998-06-01

    Within the framework of the two-center shell model the classically dynamical behaviour of a nucleon in heavy nuclei is investigated systematically with the change of nuclear shape parameters for the first time. It is found that as long as the nucleonic energy 0is appreciably higher than the height of the potential barrier there is a good quantum-classical correspondence of nucleonic regular (chaotic) motion. Thus, Bohigas, Giannoni and Schmit conjecture is confirmed once again. We find that the difference between the potential barrier for prolate nuclei and that for oblate ones is reponsible for the energy-dependence difference between the nucleonic chaotic dynamics for prolate nuclei and that for oblate ones. In addition, it is suggested that nuclear dissipation is shape-dependent, and strong nuclear dissipation can be expected for medium or large separations in the presence of a considerable neck deformation built on a pronounced octupole-like deformation, which provides us a dynamical understanding of nuclear shape dependence of nuclear dissipation. (orig.) With 5 figs., 22 refs.

  2. Performance evaluation of open core gasifier on multi-fuels

    Energy Technology Data Exchange (ETDEWEB)

    Bhoi, P.R.; Singh, R.N.; Sharma, A.M.; Patel, S.R. [Thermo Chemical Conversion Division, Sardar Patel Renewable Energy Research Institute (SPRERI), Vallabh Vidyanagar 388 120, Gujarat (India)

    2006-06-15

    Sardar Patel renewable energy research institute (SPRERI) has designed and developed open core, throat-less, down draft gasifier and installed it at the institute. The gasifier was designed for loose agricultural residues like groundnut shells. The purpose of the study is to evaluate the gasifier on multi-fuels such as babul wood (Prosopis juliflora), groundnut shell briquettes, groundnut shell, mixture of wood (Prosopis juliflora) and groundnut shell in the ratio of 1:1 and cashew nut shell. The gasifier performance was evaluated in terms of fuel consumption rate, calorific value of producer gas and gasification efficiency. Gasification efficiency of babul wood (Prosopis juliflora), groundnut shell briquettes, groundnut shell, mixture of Prosopis juliflora and groundnut shell in the ratio of 1:1 and cashew nut shell were 72%, 66%, 70%, 64%, 70%, respectively. Study revealed that babul wood (Prosopis juliflora), groundnut shell briquettes, groundnut shell, mixture of wood (Prosopis juliflora) and groundnut shell in the ratio of 1:1 and cashew nut shell were satisfactorily gasified in open core down draft gasifier. The study also showed that there was flow problem with groundnut shell. (author)

  3. Partial Dynamical Symmetries in Nuclei

    CERN Document Server

    Leviatan, A

    2000-01-01

    Partial dynamical symmetries (PDS) are shown to be relevant to the interpretation of the $K=0_2$ band and to the occurrence of F-spin multiplets of ground and scissors bands in deformed nuclei. Hamiltonians with bosonic and fermionic PDS are presented.

  4. Nuclear astrophysics of light nuclei

    DEFF Research Database (Denmark)

    Fynbo, Hans Otto Uldall

    2013-01-01

    A review of nuclear astrophysics of light nuclei using radioactive beams or techniques developed for radioactive beams is given. We discuss Big Bang nucleosynthesis, with special focus on the lithium problem, aspects of neutrino-physics, helium-burning and finally selected examples of studies...

  5. Fission dynamics of hot nuclei

    Indian Academy of Sciences (India)

    Santanu Pal; Jhilam Sadhukhan

    2014-04-01

    Experimental evidence accumulated during the last two decades indicates that the fission of excited heavy nuclei involves a dissipative dynamical process. We shall briefly review the relevant dynamical model, namely the Langevin equations for fission. Statistical model predictions using the Kramers’ fission width will also be discussed.

  6. Low energy + scattering on = nuclei

    Indian Academy of Sciences (India)

    Swapan Das; Arun K Jain

    2003-11-01

    The data for the total cross-section of + scattering on various nuclei have been analysed in the Glauber multiple scattering theory. Energy-dependent +-nucleus optical potential is generated using the forward +-nucleon scattering amplitude and the nuclear density distribution. Along with this, the calculated total +-nucleus cross-sections using the effective +-nucleon cross-section inside the nucleus are also presented.

  7. Properties and structure of N=Z nuclei within relativistic mean field theory

    Institute of Scientific and Technical Information of China (English)

    GAO Yuan; DONG Jian-Min; ZHANG Hong-Fei; ZUO Wei; LI Jun-Qing

    2009-01-01

    The axially deformed relativistic mean field theory with the force NLSH has been performed in the blocked BCS approximation to investigate the properties and structure of N=Z nuclei from Z=20 to Z=48.Some ground state quantities such as binding energies, quadrupole deformations, one/two-nucleon separation energies, root-mean-square (rms) radii of charge and neutron, and shell gaps have been calculated.The results suggest that large deformations can be found in medium-heavy nuclei with N=Z=38-42.The charge and neutron rms radii increase rapidly beyond the magic number N=Z=28 until Z=42 with increasing nucleon number, which is similar to isotope shift, yet beyond Z=42, they decrease dramatically as the structure changes greatly from Z=42 to Z=43.The evolution of shell gaps with proton number Z can be clearly observed.Besides the appearance of possible new shell closures, some conventional shell closures have been found to disappear in some region.In addition, we found that the Coulomb interaction is not strong enough to breakdown the shell structure of protons in the current region.

  8. Neutrinoless double beta nuclear matrix elements around mass 80 in the nuclear shell-model

    Science.gov (United States)

    Yoshinaga, N.; Higashiyama, K.; Taguchi, D.; Teruya, E.

    2015-05-01

    The observation of the neutrinoless double-beta decay can determine whether the neutrino is a Majorana particle or not. For theoretical nuclear physics it is particularly important to estimate three types of matrix elements, namely Fermi (F), Gamow-Teller (GT), and tensor (T) matrix elements. In this paper, we carry out shell-model calculations and also pair-truncated shell-model calculations to check the model dependence in the case of mass A=82 nuclei.

  9. Neutrinoless double beta nuclear matrix elements around mass 80 in the nuclear shell-model

    Directory of Open Access Journals (Sweden)

    Yoshinaga N.

    2015-01-01

    Full Text Available The observation of the neutrinoless double-beta decay can determine whether the neutrino is a Majorana particle or not. For theoretical nuclear physics it is particularly important to estimate three types of matrix elements, namely Fermi (F, Gamow-Teller (GT, and tensor (T matrix elements. In this paper, we carry out shell-model calculations and also pair-truncated shell-model calculations to check the model dependence in the case of mass A=82 nuclei.

  10. Recent results in quantum chaos and its applications to atomic nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Gomez, J M G; Relano, A; Retamosa, J [Departamento de Fisica Atomica, Molecular y Nuclear, Universidad Complutense de Madrid, E-28040 Madrid (Spain); Faleiro, E; Munoz, L [Departamento de Fisica Aplicada, E. U. I. T. Industrial, Universidad Politecnica de Madrid, E-28012 Madrid (Spain); Molina, R A, E-mail: gomezk@nuc1.fis.ucm.es [Instituto de Estructura de la Materia, CSIC, E-28006 Madrid (Spain)

    2011-01-01

    A survey of chaotic dynamics in atomic nuclei is presented, using on the one hand standard statistics of quantum chaos studies, and on the other a new approach based on time series analysis methods. The study of shell-model spectra in the pf shell shows that nuclear chaos is strongly isospin dependent and increases with excitation energy. On the other hand, it is found that chaotic quantum systems exhibit 1/f noise and regular systems exhibit 1/f{sup 2} behaviour. It is shown that the time series approach can be used to calculate quite accurately the fraction of missing levels and the existence of mixed symmetries in experimental level spectra.

  11. Partial dynamical symmetry in the symplectic shell model

    Energy Technology Data Exchange (ETDEWEB)

    Escher, J. [TRIUMF, Vancouver, British Columbia (Canada); Leviatan, A. [Hebrew Univ., Racah Inst. of Physics, Jerusalem (Israel)

    2000-08-01

    We present an example of a partial dynamical symmetry (PDS) in an interacting fermion system and demonstrate the close relationship of the associated Hamiltonians with a realistic quadrupole-quadrupole interaction, thus shedding light on this important interaction. Specifically, in the framework of the symplectic shell model of nuclei, we prove the existence of a family of fermionic Hamiltonians with partial SU(3) symmetry. We outline the construction process for the PDS eigenstates with good symmetry and give analytic expressions for the energies of these states and E2 transition strengths between them. Characteristics of both pure and mixed-symmetry PDS eigenstates are discussed and the resulting spectra and transition strengths are compared to those of real nuclei. The PDS concept is shown to be relevant to the description of prolate, oblate, as well as triaxially deformed nuclei. Similarities and differences between the fermion case and the previously established partial SU(3) symmetry in the interacting boson model are considered. (author)

  12. Partial Dynamical Symmetry in the Symplectic Shell Model

    CERN Document Server

    Escher, J; Escher, Jutta; Leviatan, Amiram

    2002-01-01

    We present an example of a partial dynamical symmetry (PDS) in an interacting fermion system and demonstrate the close relationship of the associated Hamiltonians with a realistic quadrupole-quadrupole interaction, thus shedding new light on this important interaction. Specifically, in the framework of the symplectic shell model of nuclei, we prove the existence of a family of fermionic Hamiltonians with partial SU(3) symmetry. We outline the construction process for the PDS eigenstates with good symmetry and give analytic expressions for the energies of these states and E2 transition strengths between them. Characteristics of both pure and mixed-symmetry PDS eigenstates are discussed and the resulting spectra and transition strengths are compared to those of real nuclei. The PDS concept is shown to be relevant to the description of prolate, oblate, as well as triaxially deformed nuclei. Similarities and differences between the fermion case and the previously established partial SU(3) symmetry in the Interact...

  13. Realistic shell model; 132Sn region; 208Pb region

    CERN Document Server

    Covello, A; Gargano, A; Itaco, N

    2008-01-01

    We report on a study of exotic nuclei around doubly magic 132Sn in terms of the shell model employing a realistic effective interaction derived from the CD-Bonn nucleon-nucleon potential. The short-range repulsion of the latter is renormalized by constructing a smooth low-momentum potential, V-low-k, that is used directly as input for the calculation of the effective interaction. In this paper, we focus attention on proton-neutron multiplets in the odd-odd nuclei 134Sb, 136Sb. We show that the behavior of these multiplets is quite similar to that of the analogous multiplets in the counterpart nuclei in the 208Pb region, 210Bi and 212Bi.

  14. Alpha decay as a probe for the structure of neutron-deficient nuclei

    CERN Document Server

    Qi, Chong

    2016-01-01

    The advent of radioactive ion beam facilities and new detector technologies have opened up new possibilities to investigate the radioactive decays of highly unstable nuclei, in particular the proton emission, $\\alpha$ decay and heavy cluster decays from neutron-deficient (or proton-rich) nuclei around the proton drip line. It turns out that these decay measurements can serve as a unique probe for studying the structure of the nuclei involved. On the theoretical side, the development in nuclear many-body theories and supercomputing facilities have also made it possible to simulate the nuclear clusterization and decays from a microscopic and consistent perspective. In this article we would like to review the current status of these structure and decay studies in heavy nuclei, regarding both experimental and theoretical opportunities. We then discuss in detail the recent progress in our understanding of the nuclear $\\alpha$ formation probabilities in heavy nuclei and their indication on the underlying nuclear st...

  15. Fast-timing studies of nuclei below $^{68}$Ni populated in the $\\beta$-decay of Mn isotopes

    CERN Multimedia

    Jokinen, A; Simpson, G S; Garcia borge, M J; Koester, U H; Georgiev, G P; Fraile prieto, L M; Aprahamian, A

    2008-01-01

    We intend to investigate structure of nuclei populated in the $\\beta$-decay of Mn isotopes via the ATD $\\beta\\gamma\\gamma$(t) technique. With this method we will measure dynamic moments in Fe isotopes and their daughters in order to characterize the role of particle-hole excitation across the ${N}$=40 sub-shell closure and the development of collectivity.

  16. An investigation of ab initio shell-model interactions derived by no-core shell model

    Science.gov (United States)

    Wang, XiaoBao; Dong, GuoXiang; Li, QingFeng; Shen, CaiWan; Yu, ShaoYing

    2016-09-01

    The microscopic shell-model effective interactions are mainly based on the many-body perturbation theory (MBPT), the first work of which can be traced to Brown and Kuo's first attempt in 1966, derived from the Hamada-Johnston nucleon-nucleon potential. However, the convergence of the MBPT is still unclear. On the other hand, ab initio theories, such as Green's function Monte Carlo (GFMC), no-core shell model (NCSM), and coupled-cluster theory with single and double excitations (CCSD), have made many progress in recent years. However, due to the increasing demanding of computing resources, these ab initio applications are usually limited to nuclei with mass up to A = 16. Recently, people have realized the ab initio construction of valence-space effective interactions, which is obtained through a second-time renormalization, or to be more exactly, projecting the full-manybody Hamiltonian into core, one-body, and two-body cluster parts. In this paper, we present the investigation of such ab initio shell-model interactions, by the recent derived sd-shell effective interactions based on effective J-matrix Inverse Scattering Potential (JISP) and chiral effective-field theory (EFT) through NCSM. In this work, we have seen the similarity between the ab initio shellmodel interactions and the interactions obtained by MBPT or by empirical fitting. Without the inclusion of three-body (3-bd) force, the ab initio shell-model interactions still share similar defects with the microscopic interactions by MBPT, i.e., T = 1 channel is more attractive while T = 0 channel is more repulsive than empirical interactions. The progress to include more many-body correlations and 3-bd force is still badly needed, to see whether such efforts of ab initio shell-model interactions can reach similar precision as the interactions fitted to experimental data.

  17. Rotating nuclei: from ground state to the extremes of spin and deformation

    CERN Document Server

    Afanasjev, A V

    2015-01-01

    The rotating nuclei represent one of most interesting subjects for theoretical and experimental studies. They open a new dimension of nuclear landscape, namely, spin direction. Contrary to the majority of nuclear systems, their properties sensitively depend on time-odd mean fields and currents in density functional theories. Moreover, they show a considerable interplay of collective and single-particle degrees of freedom. In this chapter, I discuss the basic features of the description of rotating nuclei in one-dimensional cranking approximation of covariant density functional theory. The successes of this approach to the description of rotating nuclei at low spin in pairing regime and at high spin in unpaired regime in wide range of deformations (from normal to hyperdeformation) are illustrated. I also discuss the recent progress and open questions in our understanding of the role of proton-neutron pairing in rotating nuclei at $N\\approx Z$, the physics of band termination and other phenomena in rotating nuc...

  18. Excited State Lifetime Measurements in Rare Earth Nuclei with Fast Electronics

    Science.gov (United States)

    Werner, V.; Cooper, N.; Bonett-Matiz, M.; Williams, E.; Régis, J.-M.; Rudigier, M.; Ahn, T.; Anagnostatou, V.; Berant, Z.; Bunce, M.; Elvers, M.; Heinz, A.; Ilie, G.; Jolie, J.; Radeck, D.; Savran, D.; Smith, M.

    2011-09-01

    We investigated the collectivity of the lowest excited 2+ states of even-even rare earth nuclei. The B(E2) excitation strengths of these nuclei should directly correlate to the size of the valence space, and maximize at mid-shell. The previously identified saturation of B(E2) strength in well-deformed rotors at mid-shell is put to a high precision test in this series of measurements. Lifetimes of the 2+1 states in 168Hf and 174W have been measured using the newly developed LaBr3 scintillation detectors. The excellent energy resolution in conjunction with superb time properties of the new material allows for reliable handling of background, which is a source of systematic error in such experiments. Preliminary lifetime values are obtained and discussed in the context of previous and ongoing work.

  19. Study of the effect of shell stabilization of the collective isovector valence-shell excitations along the N=80 isotonic chain

    CERN Multimedia

    It is proposed to investigate the microscopic mechanism which leads to a concentration or a fragmentation of the quadrupole-collective isovector valence-shell excitations, the so-called mixed-symmetry states (MSSs), an effect called shell stabilization of MSSs. This aim will be achieved by identification of MSSs of the unstable nuclei $^{140}$Nd and $^{142}$Sm. The first steps of this program have been undertaken in two subsequent REX-ISOLDE experiments (IS496) in which we have measured the B(E2; 2$^{+}_{1}$$\\rightarrow$ 0$^{+}_{1}$) transition strengths in the radioactive nuclei $^{140}$Nd and $^{142}$Sm. By using these data and the higher beam energy of HIE-ISOLDE we propose now to identify the MSSs of these nuclei by measuring their relative populations with respect to the population of the first 2$^{+}$ states in Coulomb excitation (CE) reactions.

  20. Scissors Mode in Gd Nuclei

    Directory of Open Access Journals (Sweden)

    Wu C.Y.

    2012-02-01

    Full Text Available Spectra of γ rays following neutron capture at isolated resonances of 6 stable Gd isotopes were measured with highly segmented BaF2 detector DANCE at the Los Alamos LANSCE spallation neutron source. The main emphasis was put on studying the γ-cascade decay of neutron resonances to get unique information on photon strength. An analysis of the accumulated γ-ray spectra within the extreme statistical model leads to an inescapable conclusion that scissors mode resonances are built not only on the ground-state, but also on excited levels in all product nuclei studied. The results on summed B(M1↑ strength and energy of the scissors mode are compared with systematics of scissors mode parameters for the ground-state transitions deduced from nuclear resonance fluorescence measurements. A specific feature of our experiments is the investigation of scissors mode of odd nuclei, for which the nuclear resonance fluorescence provides only limited information.

  1. Scissors Mode in Gd Nuclei

    Science.gov (United States)

    Kroll, J.; Baramsai, B.; Becker, J. A.; Bečvář, F.; Bredeweg, T. A.; Couture, A.; Chyzh, A.; Dashdorj, D.; Haight, R. C.; Jandel, M.; Krtička, M.; Mitchell, G. E.; O'Donnell, J. M.; Parker, W.; Rundberg, R. S.; Ullmann, J. L.; Vieira, G. J.; Walker, C. L.; Wilhelmy, J. B.; Wouters, J. M.; Wu, C. Y.

    2012-02-01

    Spectra of γ rays following neutron capture at isolated resonances of 6 stable Gd isotopes were measured with highly segmented BaF2 detector DANCE at the Los Alamos LANSCE spallation neutron source. The main emphasis was put on studying the γ-cascade decay of neutron resonances to get unique information on photon strength. An analysis of the accumulated γ-ray spectra within the extreme statistical model leads to an inescapable conclusion that scissors mode resonances are built not only on the ground-state, but also on excited levels in all product nuclei studied. The results on summed B(M1)↑ strength and energy of the scissors mode are compared with systematics of scissors mode parameters for the ground-state transitions deduced from nuclear resonance fluorescence measurements. A specific feature of our experiments is the investigation of scissors mode of odd nuclei, for which the nuclear resonance fluorescence provides only limited information.

  2. Evolution of active galactic nuclei

    CERN Document Server

    Merloni, Andrea

    2012-01-01

    [Abriged] Supermassive black holes (SMBH) lurk in the nuclei of most massive galaxies, perhaps in all of them. The tight observed scaling relations between SMBH masses and structural properties of their host spheroids likely indicate that the processes fostering the growth of both components are physically linked, despite the many orders of magnitude difference in their physical size. This chapter discusses how we constrain the evolution of SMBH, probed by their actively growing phases, when they shine as active galactic nuclei (AGN) with luminosities often in excess of that of the entire stellar population of their host galaxies. Following loosely the chronological developments of the field, we begin by discussing early evolutionary studies, when AGN represented beacons of light probing the most distant reaches of the universe and were used as tracers of the large scale structure. This early study turned into AGN "Demography", once it was realized that the strong evolution (in luminosity, number density) of ...

  3. Proton scattering from unstable nuclei

    Indian Academy of Sciences (India)

    Y Blumenfeld; E Khan; F Maréchal; T Suomijärvi

    2001-08-01

    Recent improvements in the intensities and optical qualities of radioactive beams have made possible the study of elastic and inelastic proton scattering on unstable nuclei. The design and performances of an innovative silicon strip detector array devoted to such experiments are described. The quality of the data obtained are illustrated with recent results obtained at the GANIL facility for unstable oxygen, sulfur and argon isotopes. Methods to analyse the data using phenomenological and microscopic optical model potentials are discussed.

  4. Weak pion production from nuclei

    Indian Academy of Sciences (India)

    S K Singh; M Sajjad Athar; Shakeb Ahmad

    2006-04-01

    The charged current pion production induced by neutrinos in 12C, 16O and 56Fe nuclei has been studied. The calculations have been done for the coherent as well as the incoherent processes assuming dominance and takes into account the effect of Pauli blocking, Fermi motion and the renormalization of in the nuclear medium. The pion absorption effects have also been taken into account.

  5. Double pion photoproduction in nuclei

    CERN Document Server

    Vicente-Vacas, M J; Gómez-Tejedor, J A; Vicente-Vacas, M J; Oset, E; Gómez Tejedor, J A

    1994-01-01

    Abstract: The inclusive A(gamma,pi+ pi-)X reaction is studied theoretically. A sizeable enhancement of the cross section is found, in comparison with the scaling of the deuteron cross section (sigma_deuteron * A/2). This enhancement is due to the modifications in the nuclear medium of the gamma N ----> pi pi N amplitude and the pion dispersion relation. The enhancement is found to be bigger than the one already observed in the (pi,pi pi) reaction in nuclei.

  6. Continuum spectroscopy of light nuclei

    Directory of Open Access Journals (Sweden)

    Charity R. J.

    2016-01-01

    Full Text Available Resonance spectroscopy of light nuclei is discussed with emphasis on the invariant-mass measurements performed with the HiRA detector. For three-body exit channels, we consider the exact conditions necessary such that the decay can be described as either sequential or prompt. However experimentally, we find some cases where the decay is intermediate between these two limits. Finally, two-proton decay from isobaric analog states is discussed.

  7. Geometric symmetries in light nuclei

    CERN Document Server

    Bijker, Roelof

    2016-01-01

    The algebraic cluster model is is applied to study cluster states in the nuclei 12C and 16O. The observed level sequences can be understood in terms of the underlying discrete symmetry that characterizes the geometrical configuration of the alpha-particles, i.e. an equilateral triangle for 12C, and a regular tetrahedron for 16O. The structure of rotational bands provides a fingerprint of the underlying geometrical configuration of alpha-particles.

  8. Dynamical effects in fusion with exotic nuclei

    Science.gov (United States)

    Vo-Phuoc, K.; Simenel, C.; Simpson, E. C.

    2016-08-01

    Background: Reactions with stable beams have demonstrated strong interplay between nuclear structure and fusion. Exotic beam facilities open new perspectives to understand the impact of neutron skin, large isospin, and weak binding energies on fusion. Microscopic theories of fusion are required to guide future experiments. Purpose: To investigate new effects of exotic structures and dynamics in near-barrier fusion with exotic nuclei. Method: Microscopic approaches based on the Hartree-Fock (HF) mean-field theory are used for studying fusion barriers in -54Ca40+116Sn reactions for even isotopes. Bare potential barriers are obtained assuming frozen HF ground-state densities. Dynamical effects on the barrier are accounted for in time-dependent Hartree-Fock (TDHF) calculations of the collisions. Vibrational couplings are studied in the coupled-channel framework and near-barrier nucleon transfer is investigated with TDHF calculations. Results: The development of a neutron skin in exotic calcium isotopes strongly lowers the bare potential barrier. However, this static effect is not apparent when dynamical effects are included. On the contrary, a fusion hindrance is observed in TDHF calculations with the most neutron-rich calcium isotopes which cannot be explained by vibrational couplings. Transfer reactions are also important in these systems due to charge equilibration processes. Conclusions: Despite its impact on the bare potential, the neutron skin is not seen as playing an important role in the fusion dynamics. However, the charge transfer with exotic projectiles could lead to an increase of the Coulomb repulsion between the fragments, suppressing fusion. The effects of transfer and dissipative mechanisms on fusion with exotic nuclei deserve further studies.

  9. Study of neutron-rich nuclei using deep-inelastic reactions

    Energy Technology Data Exchange (ETDEWEB)

    Lee, I.Y.; Asztalos, S.; Deleplanque, M.; Cederwall, B.; Diamond, R.M.; Fallon, P.; Macchiavelli, A.O.; Phair, L.; Stephens, F.S.; Wozniak, G.J. [Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Frauendorf, S.G. [Research Center Rossendorf, Dresden (Germany); Becker, J.A.; Henry, E.A. [Lawrence Livermore National Laboratory, Livermore, California 94550 (United States); Hua, P.F.; Sarantites, D.G. [Washington University, St. Louis, Missouri 63130 (United States); Saladin, J.X. [University of Pittsburgh, Pittsburgh, Pennsylvania 15260 (United States); Yu, C.H. [University of Rochester, Rochester, New York 14627 (United States)

    1997-08-01

    We have used the {sup 48}Ca+{sup 176}Yb reaction to study the population of high-spin states in neutron-rich nuclei by deep-inelastic reactions. Using Gammasphere, we observed gamma transitions from nuclei several neutrons richer than the target. Yrast states with spin up to 20 were populated in this reaction. High-spin states in {sup 175,177,178}Yb were observed. In this region of reduced pairing, a reference based on experimental data was used to derive experimental Routhians. Systematics of experimental Routhians in neutron-rich Yb nuclei compare well with cranked shell-model calculations. {copyright} {ital 1997} {ital The American Physical Society}

  10. Emergent properties of nuclei from ab initio coupled-cluster calculations

    CERN Document Server

    Hagen, G; Hjorth-Jensen, M; Papenbrock, T

    2016-01-01

    Emergent properties such as nuclear saturation and deformation, and the effects on shell structure due to the proximity of the scattering continuum and particle decay channels are fascinating phenomena in atomic nuclei. In recent years, ab initio approaches to nuclei have taken the first steps towards tackling the computational challenge of describing these phenomena from Hamiltonians with microscopic degrees of freedom. This endeavor is now possible due to ideas from effective field theories, novel optimization strategies for nuclear interactions, ab initio methods exhibiting a soft scaling with mass number, and ever-increasing computational power. This paper reviews some of the recent accomplishments. We also present new results. The recently optimized chiral interaction NNLO$_{\\rm sat}$ is shown to provide an accurate description of both charge radii and binding energies in selected light- and medium-mass nuclei up to $^{56}$Ni. We derive an efficient scheme for including continuum effects in coupled-clust...

  11. A statistical approach to describe highly excited heavy and superheavy nuclei

    Science.gov (United States)

    Chen, Peng-Hui; Feng, Zhao-Qing; Li, Jun-Qing; Zhang, Hong-Fei

    2016-09-01

    A statistical approach based on the Weisskopf evaporation theory has been developed to describe the de-excitation process of highly excited heavy and superheavy nuclei, in particular for the proton-rich nuclei. The excited nucleus is cooled by evaporating γ-rays, light particles (neutrons, protons, α etc) in competition with binary fission, in which the structure effects (shell correction, fission barrier, particle separation energy) contribute to the processes. The formation of residual nuclei is evaluated via sequential emission of possible particles above the separation energies. The available data of fusion-evaporation excitation functions in the 28Si+198Pt reaction can be reproduced nicely within the approach. Supported by Major State Basic Research Development Program in China (2015CB856903), National Natural Science Foundation of China Projects (11175218, U1332207, 11475050, 11175074), and Youth Innovation Promotion Association of Chinese Academy of Sciences

  12. Effects of thermal shape fluctuations and pairing fluctuations on the giant dipole resonance in warm nuclei

    CERN Document Server

    Kumar, A K Rhine; Dang, N Dinh

    2015-01-01

    Apart from the higher limits of isospin and temperature, the properties of atomic nuclei are intriguing and less explored at the limits of lowest but finite temperatures. At very low temperatures there is a strong interplay between the shell (quantal fluctuations), statistical (thermal fluctuations), and residual pairing effects as evidenced from the studies on giant dipole resonance (GDR). In our recent work [Phys. Rev. C \\textbf{90}, 044308 (2014)], we have outlined some of our results from a theoretical approach for such warm nuclei where all these effects are incorporated along within the thermal shape fluctuation model (TSFM) extended to include the fluctuations in the pairing field. In this article, we present the complete formalism based on the microscopic-macroscopic approach for determining the deformation energies and a macroscopic approach which links the deformation to GDR observables. We discuss our results for the nuclei $^{97}$Tc, $^{120}$Sn, $^{179}$Au, and $^{208}$Pb, and corroborate with the...

  13. Influence of Isotope on Shell Effects of Pre-scission Particle Evaporation

    Institute of Scientific and Technical Information of China (English)

    YE Wei; CHEN Na

    2005-01-01

    The shell effects on the particle evaporation prior to fission for three Pb isotopes, 204pb, 20sPb, and 212pb,as well as three Sn isotopes, 128Sn, 132Sn, and 136Sn, are explored by a diffusion model. Calculations show that the magnitude of shell effects in the emission of particles changes with the neutron-to-proton ratio N/Z of these fissioning nuclei, and this change is affected significantly by the spin and excitation energy of the system. It is shown that high angular momentum enhances the dependence of shell effects on the N/Z while high excitation energy weakens such a dependence.

  14. No influence of a N=126 Neutron Shell Closure in Fission Fragment Mass Distributions

    CERN Document Server

    Chaudhuri, A; Banerjee, K; Bhattacharya, S; Sadhukhan, Jhilam; Kundu, S; Bhattacharya, C; Meena, J K; Mukherjee, G; Saha, A K; Asgar, Md A; Dey, A; Manna, S; Pandey, R; Rana, T K; Roy, P; Roy, T; Srivastava, V; Bhattacharya, P; Biswas, D C; Joshi, B N; Mahata, K; Shrivastava, A; Vind, R P; Pal, S; Behera, B R; Singh, Varinderjit

    2015-01-01

    Mass distributions of the fragments in the fission of $^{206}$Po and the N=126 neutron shell closed nucleus $^{210}$Po have been measured. No significant deviation of mass distributions has been found between $^{206}$Po and $^{210}$Po, indicating the absence of shell correction at the saddle point in both the nuclei, contrary to the reported angular anisotropy and pre-scission neutron multiplicity results. This new result provides benchmark data to test the new fission dynamical models to study the effect of shell correction on the potential energy surface at saddle point.

  15. Precise comparison of the Gaussian expansion method and the Gamow shell model

    CERN Document Server

    Masui, Hiroshi; Michel, Nicola; Płoszajczak, Marek

    2014-01-01

    We perform a detailed comparison of results of the Gamow Shell Model (GSM) and the Gaussian Expansion Method (GEM) supplemented by the complex scaling (CS) method for the same translationally-invariant cluster-orbital shell model (COSM) Hamiltonian. As a benchmark test, we calculate the ground state $0^{+}$ and the first excited state $2^{+}$ of mirror nuclei $^{6}$He and $^{6}$Be in the model space consisting of two valence nucleons in $p$-shell outside of a $^{4}$He core. We find a good overall agreement of results obtained in these two different approaches, also for many-body resonances.

  16. GALS – setup for production and study of heavy neutron rich nuclei

    CERN Document Server

    Zemlyanoy, Sergey; Kozulin, Eduard; Kudryavtsev, Yury; Fedosseev, Valentin; Bark, Robert; Janas, Zenon; Othman, Hosam

    2015-01-01

    The present limits of the upper part of the nuclear map are very close to stability while the unexplored area of heavy neutron-rich nuclides along the neutron closed shell N = 126 below ^208Pb is extremely important for nuclear astrophysics investigations and, in particular, for the understanding of the r-process of astrophysical nucleosynthesis. This area of the nuclear map can be reached neither in fusion-fission reactions nor in fragmentation processes widely used nowadays for the production of exotic nuclei. A new way was recently proposed for the production of these nuclei via low-energy multi-nucleon transfer reactions. The estimated yields of neutron-rich nuclei are found to be significantly high in such reactions and several tens of new nuclides can be produced, for example, in the near-barrier collision of ^136Xe with ^208Pb. A new setup is proposed to produce and study heavy neutron-rich nuclei located along the neutron closed shell N=126.

  17. GALS – setup for production and study of heavy neutron rich nuclei

    Directory of Open Access Journals (Sweden)

    Zemlyanoy Sergey

    2015-01-01

    Full Text Available The present limits of the upper part of the nuclear map are very close to stability while the unexplored area of heavy neutron-rich nuclides along the neutron closed shell N = 126 below 208Pb is extremely important for nuclear astrophysics investigations and, in particular, for the understanding of the r-process of astrophysical nucleosynthesis. This area of the nuclear map can be reached neither in fusion–fission reactions nor in fragmentation processes widely used nowadays for the production of exotic nuclei. A new way was recently proposed for the production of these nuclei via low-energy multi-nucleon transfer reactions. The estimated yields of neutron-rich nuclei are found to be significantly high in such reactions and several tens of new nuclides can be produced, for example, in the near-barrier collision of 136Xe with 208Pb. A new setup is proposed to produce and study heavy neutron-rich nuclei located along the neutron closed shell N=126.

  18. Elastic platonic shells.

    Science.gov (United States)

    Yong, Ee Hou; Nelson, David R; Mahadevan, L

    2013-10-25

    On microscopic scales, the crystallinity of flexible tethered or cross-linked membranes determines their mechanical response. We show that by controlling the type, number, and distribution of defects on a spherical elastic shell, it is possible to direct the morphology of these structures. Our numerical simulations show that by deflating a crystalline shell with defects, we can create elastic shell analogs of the classical platonic solids. These morphologies arise via a sharp buckling transition from the sphere which is strongly hysteretic in loading or unloading. We construct a minimal Landau theory for the transition using quadratic and cubic invariants of the spherical harmonic modes. Our approach suggests methods to engineer shape into soft spherical shells using a frozen defect topology.

  19. β -Decay Half-Lives of 110 Neutron-Rich Nuclei across the N=82 Shell Gap: Implications for the Mechanism and Universality of the Astrophysical r Process

    Energy Technology Data Exchange (ETDEWEB)

    Lorusso, G.; Nishimura, S.; Xu, Z. Y.; Jungclaus, A.; Shimizu, Y.; Simpson, G. S.; Söderström, P. -A.; Watanabe, H.; Browne, F.; Doornenbal, P.; Gey, G.; Jung, H. S.; Meyer, B.; Sumikama, T.; Taprogge, J.; Vajta, Zs.; Wu, J.; Baba, H.; Benzoni, G.; Chae, K. Y.; Crespi, F. C. L.; Fukuda, N.; Gernhäuser, R.; Inabe, N.; Isobe, T.; Kajino, T.; Kameda, D.; Kim, G. D.; Kim, Y. -K.; Kojouharov, I.; Kondev, F. G.; Kubo, T.; Kurz, N.; Kwon, Y. K.; Lane, G. J.; Li, Z.; Montaner-Pizá, A.; Moschner, K.; Naqvi, F.; Niikura, M.; Nishibata, H.; Odahara, A.; Orlandi, R.; Patel, Z.; Podolyák, Zs.; Sakurai, H.; Schaffner, H.; Schury, P.; Shibagaki, S.; Steiger, K.; Suzuki, H.; Takeda, H.; Wendt, A.; Yagi, A.; Yoshinaga, K.

    2015-05-01

    The β -decay half-lives of 110 neutron-rich isotopes of the elements from Rb 37 to Sn 50 were measured at the Radioactive Isotope Beam Factory. The 40 new half-lives follow robust systematics and highlight the persistence of shell effects. The new data have direct implications for r -process calculations and reinforce the notion that the second (A≈130 ) and the rare-earth-element (A≈160 ) abundance peaks may result from the freeze-out of an (n,γ)⇌(γ,n) equilibrium. In such an equilibrium, the new half-lives are important factors determining the abundance of rare-earth elements, and allow for a more reliable discussion of the r process universality. It is anticipated that universality may not extend to the elements Sn, Sb, I, and Cs, making the detection of these elements in metal-poor stars of the utmost importance to determine the exact conditions of individual r -process events.

  20. Partial Dynamical Symmetry in the f7/2 and g9/2 shell

    CERN Document Server

    Zamick, Larry

    2011-01-01

    We discuss partial dynamical symmetries which occur in single j shell calculations mostly for high spin states for systems of three or four particles (holes). The relevant nuclei are 43Ti,43Sc, 44Ti, 52Fe,53Fe, 53Co,96Cd,97Cd, and 97In.

  1. Shell model study of $^{40}$Ca muon capture and the $(0^+, 0)

    CERN Document Server

    Gorringe, T P

    2006-01-01

    We report results from shell model studies of muon capture on $^{40}$Ca to low-lying levels of $^{40}$K. We discuss the comparison between calculated capture rates, measured capture rates and analogous transitions in ($e$,$e^{\\prime}$) scattering in terms of the particle-hole structure of the $^{40}$Ca-$^{40}$K nuclei. We highlight the $^{40}$Ca$(0^+, 0)

  2. Three-cluster model for the α-accompanied fission of californium nuclei

    Science.gov (United States)

    Manimaran, K.; Balasubramaniam, M.

    2009-02-01

    A three-cluster model is proposed to explain the particle-accompanied binary fission of radioactive nuclei. The model is developed as an extension of the preformed cluster model of Gupta and collaborators. The advantage of this model is that, for a fixed third fragment, we can calculate the fragmentation potential minimized in charge coordinate. For our study we chose the various neutron-deficient to neutron-rich californium nuclei, whose analysis reveals that the closed-shell effect of any one of the fragments in ternary fragmentation presents itself as the most favorable configuration to be observed. As one goes from a neutron-deficient to a neutron-rich californium isotope, the role of the neutron closed shell associated with any one of the preferred fragments changes to that of the proton closed shell, and for very neutron rich isotopes of californium the presence of a double closed shell nucleus enhances the decay probability. The quadrupole deformation of the light fragment (A2) associated with the preferred configuration in the symmetric mass region also has a transition from positive to negative deformation as one goes from neutron-deficient to neutron-rich californium isotopes. The calculated relative yields of different fragmentation channels are compared with the available experimental yields for Cf252.

  3. New Generation of the Monte Carlo Shell Model for the K Computer Era

    CERN Document Server

    Shimizu, Noritaka; Tsunoda, Yusuke; Utsuno, Yutaka; Yoshida, Tooru; Mizusaki, Takahiro; Honma, Michio; Otsuka, Takaharu

    2012-01-01

    We present a newly enhanced version of the Monte Carlo Shell Model method by incorporating the conjugate gradient method and energy-variance extrapolation. This new method enables us to perform large-scale shell-model calculations that the direct diagonalization method cannot reach. This new generation framework of the MCSM provides us with a powerful tool to perform most-advanced large-scale shell-model calculations on current massively parallel computers such as the K computer. We discuss the validity of this method in ab initio calculations of light nuclei, and propose a new method to describe the intrinsic wave function in terms of the shell-model picture. We also apply this new MCSM to the study of neutron-rich Cr and Ni isotopes using the conventional shell-model calculations with an inert 40Ca core and discuss how the magicity of N = 28, 40, 50 remains or is broken.

  4. Tensor Effect on Bubble Nuclei

    Institute of Scientific and Technical Information of China (English)

    WANG Yan-Zhao; GU Jian-Zhong; ZHANG Xi-Zhen; DONG Jian-Min

    2011-01-01

    In the framework of the Hartree-Fock-Bogoliubov (HFB) approach with Skyrme interactions SLy5+T, SLy5+Tw and several sets of TIJ parametrizations, I.e. The Skyrme interaction parametrizations including the tensor terms, the proton density distribution in 34Si and 46Ar nuclei is calculated with and without the tensor force. It is shown that the bubble effect in 34Si does not depend a great deal on the Skyrme parametrization and the proton density distribution in 34Si is hardly influenced by the tensor force. As to 46Ar, the SLy5+Tw parametrization favors the formation of the bubble structure due to the inversion between the 2s1/2 and 1d3/2 orbits (2s1/2-ld3/2 inversion). The inversion mechanism induced by the SLy5+Tw interaction is analyzed based on the proton single-particle spectra obtained from the SLy5 and SLy5+Tw interactions as well as the wave functions of the 2s1/2 and 1d3/2 states.%In the framework of the Hartree-Fock-Bogoliubov (HFB) approach with Skyrme interactions SLy5+ T,SLy5+ Tω and several sets of TIJ parametrizations,i.e.the Skyrme interaction pararmetrizations including the tensor terms,the proton density distribution in 34Si and 46 Ar nuclei is calculated with and without the tensor force.It is shown that the bubble effect in 34Si does not depend a great deal on the Skyrme parametrization and the proton density distribution in 34Si is hardly influenced by the tensor force.As to 46Ar,the SLy5+ Tω parametrization favors the formation of the bubble structure due to the inversion between the 2s1/2 and 1d3/2 orbits (2s1/2-1d3/2 inversion).The inversion mechanism induced by the SLy5+ Tω interaction is analyzed based on the proton single-particle spectra obtained from the SLy5 and SLy5+ Tω interactions as well as the wave functions of the 2s1/2 and 1d3/2 states.The study of exotic nuclear structures has been a hot topic in nuclear physics.[1-4] Exotic nuclei are unstabile,superheavy nuclei,halo nuclei and so forth,whose structures are quite different

  5. Multi-Shell Hollow Nanogels with Responsive Shell Permeability.

    Science.gov (United States)

    Schmid, Andreas J; Dubbert, Janine; Rudov, Andrey A; Pedersen, Jan Skov; Lindner, Peter; Karg, Matthias; Potemkin, Igor I; Richtering, Walter

    2016-03-17

    We report on hollow shell-shell nanogels with two polymer shells that have different volume phase transition temperatures. By means of small angle neutron scattering (SANS) employing contrast variation and molecular dynamics (MD) simulations we show that hollow shell-shell nanocontainers are ideal systems for controlled drug delivery: The temperature responsive swelling of the inner shell controls the uptake and release, while the thermoresponsive swelling of the outer shell controls the size of the void and the colloidal stability. At temperatures between 32 °C shell. Computer simulations showed, that temperature induced switching of the permeability of the inner shell allows for the encapsulation in and release of molecules from the cavity.

  6. Confocal Raman spectroscopy of island nuclei formed at the initial stage of quartz glass crystallization

    Science.gov (United States)

    Pankin, D. V.; Zolotarev, V. M.; Colas, M.; Cornette, J.; Evdokimova, M. G.

    2016-12-01

    Island nuclei formed on a polished quartz-glass surface upon heating to 1100°C have been investigated by confocal Raman spectroscopy. The structural and chemical composition of islands is shown to be a central nucleus, a shell around the nucleus, and a thin peripheral ring closing this shell. The formation and growth of individual regions of an island nucleus are found to occur in several stages. The shell around the nucleus is mainly formed by α-SiO2 and α-cristobalite nanoparticles with a size ≥40 nm, whereas the α-SiO2 nanoparticles in the nucleus and peripheral ring are 2-15 nm in size.

  7. Calculation of α preformation for nuclei near N=162 and N=184

    Science.gov (United States)

    Zhang, G. L.; Le, X. Y.; Zhang, H. Q.

    2009-12-01

    The α preformation factor and the penetration probability are carefully analyzed for heavy and superheavy even-even nuclei. The penetration probability of an α cluster in the parent nucleus is calculated within the WKB approximation, whereas the nuclear potential between an α cluster and the daughter nucleus is obtained in the frame of a double-folding model with a density-dependent nucleon-nucleon interaction, in which the zero-range exchange term is supplemented. The α preformation factors in different shell regions are compared. It is shown that shell effects play an important role in α preformation. The preformation factor can supply information on the nuclear structure, and the penetration probability mainly determines the α-decay half-life. The results indicate that the deformed-subshell region at N=162 is different from that at N=152, and Z=114 and N=184 may lie in the closed-shell region.

  8. Deformed configurations, band structures and spectroscopic properties of = 50 Ge and Se nuclei

    Indian Academy of Sciences (India)

    S K Ghorui; C R Praharaj

    2014-04-01

    The deformed configurations and rotational band structures in =50 Ge and Se nuclei are studied by deformed Hartree–Fock with quadrupole constraint and angular momentum projection. Apart from the `almost’ spherical HF solution, a well-deformed configuration occurs at low excitation. A deformed well-mixed = 1/2+ neutron orbit comes down in energy (from the shell above = 50) to break the = 50 spherical shell closure. A = 7− isomer is predicted in 84Se at fairly low excitation energy. At higher excitation energies (8 MeV), a deformed band with = 7/2+–1/2− (based on $h_{11/2}$) neutron 1p–1h excitation, for 82Ge and 84Se, is shown in our calculation. Our study gives insight into possible deformed structures at spherical shell closure.

  9. “A STUDY ON SECURE SHELL (SSH PROTOCOL”

    Directory of Open Access Journals (Sweden)

    NIDHI KANDHIL

    2011-08-01

    Full Text Available Secure Shell (SSH provides an open protocol for securing network communications that is less complex and expensive than hardware-based VPN solutions. Secure Shell client/server solutions provide command shell, file transfer, and data tunneling services for TCP/IP applications. SSH connections provide highly secure authentication, encryption, and data integrity to combat password theft and other security threats. VanDyke Software® clients and servers are mature native Windows implementations that offer a range of SSH apabilities and are interoperable with SSH software on other platforms.

  10. Three-body halo nuclei in an effective theory framework

    Energy Technology Data Exchange (ETDEWEB)

    Canham, David L.

    2009-05-20

    The universal properties and structure of halo nuclei composed of two neutrons (2n) and a core are investigated within an effective quantum mechanics framework. We construct an effective interaction potential that exploits the separation of scales in halo nuclei and treat the nucleus as an effective three-body system, which to leading order is described by the large S-wave scattering lengths in the underlying two-body subsystems. The uncertainty from higher orders in the expansion is quantified through theoretical error bands. First, we investigate the possibility to observe excited Efimov states in 2n halo nuclei. Based on the experimental data, {sup 20}C is the only halo nucleus candidate to possibly have an Efimov excited state, with an energy less than 7 keV below the scattering threshold. Second, we study the structure of {sup 20}C and other 2n halo nuclei. In particular, we calculate their matter density form factors, radii, and two-neutron opening angles. We then make a systematic improvement upon these calculations by extending the effective potential to the next-to-leading order. To this order, we require an additional two-body parameter, which we tune to the effective range of the interaction. In addition to range corrections to the 2n halo nuclei results, we show corrections to the Efimov effect in the three-boson system. Furthermore, we explore universality in the linear range corrections to the Efimov spectrum. Finally, we study the scattering of D{sup 0} and D{sup *0} mesons and their antiparticles off the X(3872) in an effective field theory for short-range interactions. We present results for the S-wave scattering amplitude, total interaction cross section and S-wave scattering length. (orig.)

  11. Multipole strength function of deformed superfluid nuclei made easy

    CERN Document Server

    Stoitsov, M; Nakatsukasa, T; Losa, C; Nazarewicz, W

    2011-01-01

    We present an efficient method for calculating strength functions using the finite amplitude method (FAM) for deformed superfluid heavy nuclei within the framework of the nuclear density functional theory. We demonstrate that FAM reproduces strength functions obtained with the fully self-consistent quasi-particle random-phase approximation (QRPA) at a fraction of computational cost. As a demonstration, we compute the isoscalar and isovector monopole strength for strongly deformed configurations in $^{240}$Pu by considering huge quasi-particle QRPA spaces. Our approach to FAM, based on Broyden's iterative procedure, opens the possibility for large-scale calculations of strength distributions in well-bound and weakly bound nuclei across the nuclear landscape.

  12. Fission of super-heavy nuclei explored with Skyrme forces

    CERN Document Server

    Schindzielorz, N; Klüpfel, P; Reinhard, P -G; Hager, G

    2010-01-01

    We present a large scale survey of life-times for spontaneous fission in the regime of super-heavy elements (SHE), i.e. nuclei with Z=104-122. This is done on the basis of the Skyrme-Hartree-Fock model. The axially symmetric fission path is computed using a quadrupole constraint. Self-consistent cranking is used for the collective masses and associated quantum corrections. The actual tunneling probability is estimated by the WKB approximation. Three typical Skyrme forces are used to explore the sensitivity of the results. Benchmarks in the regime Z=104-108 show an acceptable agreement. The general systematics reflects nicely the islands of shell stabilization and the crossover from $\\alpha$-decay to fission for the decay chains from the region of Z/N=118/176.

  13. Remarks on the fission barriers of super-heavy nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Hofmann, S. [GSI Helmholtzzentrum fuer Schwerionenforschung, Darmstadt (Germany); Goethe-Universitaet Frankfurt, Institut fuer Physik, Frankfurt (Germany); Heinz, S.; Mann, R.; Maurer, J.; Muenzenberg, G.; Barth, W.; Dahl, L.; Kindler, B.; Kojouharov, I.; Lang, R.; Lommel, B.; Runke, J.; Scheidenberger, C.; Tinschert, K. [GSI Helmholtzzentrum fuer Schwerionenforschung, Darmstadt (Germany); Antalic, S. [Comenius University, Department of Nuclear Physics and Biophysics, Bratislava (Slovakia); Eberhardt, K.; Thoerle-Pospiech, P.; Trautmann, N. [Johannes Gutenberg-Universitaet Mainz, Mainz (Germany); Grzywacz, R. [Oak Ridge National Laboratory, Oak Ridge, TN (United States); University of Tennessee, Knoxville, TN (United States); Hamilton, J.H. [Vanderbilt University, Department of Physics and Astronomy, Nashville, TN (United States); Henderson, R.A.; Kenneally, J.M.; Moody, K.J.; Shaughnessy, D.A.; Stoyer, M.A. [Lawrence Livermore National Laboratory, Livermore, CA (United States); Miernik, K. [Oak Ridge National Laboratory, Oak Ridge, TN (United States); University of Warsaw, Warsaw (Poland); Miller, D. [University of Tennessee, Knoxville, TN (United States); Morita, K. [RIKEN Nishina Center for Accelerator-Based Science, Wako, Saitama (Japan); Nishio, K. [Japan Atomic Energy Agency, Tokai, Ibaraki (Japan); Popeko, A.G.; Yeremin, A.V. [Joint Institute for Nuclear Research, Dubna (Russian Federation); Roberto, J.B.; Rykaczewski, K.P. [Oak Ridge National Laboratory, Oak Ridge, TN (United States); Uusitalo, J. [University of Jyvaeskylae, Department of Physics, Jyvaeskylae (Finland)

    2016-04-15

    Shell-correction energies of super-heavy nuclei are approximated by using Q{sub α} values of measured decay chains. Five decay chains were analyzed, which start at the isotopes {sup 285}Fl, {sup 294}118, {sup 291}Lv, {sup 292}Lv and {sup 293}Lv. The data are compared with predictions of macroscopic-microscopic models. Fission barriers are estimated that can be used to eliminate uncertainties in partial fission half-lives and in calculations of evaporation-residue cross-sections. In that calculations, fission probability of the compound nucleus is a major factor contributing to the total cross-section. The data also provide constraints on the cross-sections of capture and quasi-fission in the entrance channel of the fusion reaction. Arguments are presented that fusion reactions for synthesis of isotopes of elements 118 and 120 may have higher cross-sections than assumed so far. (orig.)

  14. Inner Radiation Belt Generation of Light Nuclei Isotope

    Science.gov (United States)

    Galper, A. M.; Koldashov, S. V.; Leonv, A. A.; Mikhailov, V. V.

    2003-07-01

    Nuclear interactions between inner zone protons and atoms in the upper atmosphere provide the essential source of H and He isotop es nuclei in radiation belt. This paper reports the calculations of these isotop es intensities from the inner zone proton intensity model AP-8, the atmosphere drift-averaged composition and densities model MSIS-90, and cross sections for the various interaction processes. To calculate drift-averaged densities and energy losses of secondaries the particles are traced in geomagnetic field according IGRF-95 model by numerical solution of motion equation. The calculations account for nuclear interactions kinematic along the whole trapped protons trajectories. The results of calculations are compared with experimental data from SAMPEX, CRRES, RESURS-04 and MITA satellites taken during different solar activity phases. The comparison with observational data shows that the atmosphere is sufficient source for inner zone 4 He, 3 He,2 H and 3 H for L-shell less than 1.3.

  15. α-decay half-lives in medium mass nuclei

    Science.gov (United States)

    Qian, Yibin; Ren, Zhongzhou; Ni, Dongdong

    2011-01-01

    Systematical calculations on the α-decay half-lives of even-even medium mass nuclei with 82 cluster model using a two-potential approach. The decay width is achieved in terms of the bound state wavefunction, the scattering wavefunction and the outer potential, where the effective α-nucleus potential is obtained from the double-folded integral of the realistic nucleon-nucleon interaction with the mass distributions of α particle and daughter nucleus. Instead of the Wentzel-Kramers-Brillouin (WKB) barrier penetration probability, the numerical solution of the Schrödinger equation for the bound state is presented. In addition, the shell effect on the α-preformation factor has been taken into account for even-even N = 126 isotones. The calculated α-decay half-lives are found to agree with experimental data with a mean factor of less than 2.

  16. Microscopic properties of superdeformed nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Karlsson, Lennart B

    1999-04-01

    Many high spin rotational bands in superdeformed nuclei have been found in the A 140 - 150 region, but so far no linking transitions to known normal-deformed states have been found in these nuclei. Therefore, configuration and spin assignments have to be based on indirect spectroscopic information. Identical bands were first discovered in this region of superdeformed states. At present, some identical bands have also been found at normal deformation, but such bands are more common at superdeformation. Recently lifetime measurements have given relative quadrupole moments with high accuracy. Spectroscopic quantities are calculated using the configuration constrained cranked Nilsson-Strutinsky model with the modified oscillator potential. In a statistical study the occurrence of identical bands is tested. Comparing superdeformed and normal deformed nuclei, the higher possibility for identical bands at superdeformation is understood from calculated reduced widths of the E{sub {gamma}} and J{sup (2)} distributions. The importance of high-N orbitals for identical bands is also discussed. Additivity of electric quadrupole moment contributions in the superdeformed A - 150 region is discussed with the nucleus {sup 152}Dy as a `core`. In analytic harmonic oscillator calculations, the effective electric quadrupole moment q{sub eff}, i.e. the change in the total quadrupole moment caused by the added particle, is expressed as a simple function of the single-particle mass, quadrupole moment q{sub {nu}}. Also in realistic calculations, simple relations between q{sub eff} and q{sub {nu}} can be used to estimate the total electric quadrupole moment, e.g. for the nucleus {sup 142}Sm, by adding the effect of 10 holes, to the total electric quadrupole moment of {sup 152}Dy. Furthermore, tools are given for estimating the quadrupole moment for possible configurations in the superdeformed A - 150 region. For the superdeformed region around {sup 143}Eu, configuration and spin assignments

  17. Breakup Densities of Hot Nuclei.

    Science.gov (United States)

    Viola, Vic

    2006-04-01

    Breakup densities of hot ^197Au-like residues have been deduced from the systematic trends of Coulomb parameters required to fit intermediate-mass-fragment kinetic-energy spectra. The results indicate emission from nuclei near normal nuclear density below an excitation energy E*/A .3ex˜x 5 MeV. Temperatures derived from these data with a density-dependent Fermi-gas model yield a nuclear caloric curve that is generally consistent with those derived from isotope ratios.

  18. Double pion photoproduction in nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Gomez Tejedor, J.A. [Departamento de Fisica Teorica, Valencia (Spain); Vicente-Vacas, M.J. [Departamento de Fisica Teorica, Valencia (Spain); Oset, E. [Departamento de Fisica Teorica, Valencia (Spain)

    1995-06-19

    The inclusive A({gamma},{pi}{sup +}{pi}{sup -})X reaction is studied theoretically. A sizable enhancement of the cross section is found, in comparison with the scaling of the deuteron cross section ({sigma}{sub d} A/2). This enhancement is due to the modifications in the nuclear medium of the {gamma}N {yields}{pi}{pi}N amplitude and the pion dispersion relation. The enhancement is found to be bigger than the one already observed in the ({pi},{pi}{pi}) reaction in nuclei. ((orig.)).

  19. Theoretical predictions on the decay properties of superheavy nuclei Z = 123 in the region 297 ≤ A ≤ 307

    Science.gov (United States)

    Santhosh, K. P.; Nithya, C.

    2016-12-01

    Decay modes of isotopes of the superheavy element Z = 123 within the range 297 ≤ A ≤ 307 have been studied by comparing the alpha decay half-lives with the spontaneous fission half-lives. Three different mass tables were used for the calculation of the alpha decay energy. A close study of alpha decay half-lives within the range 297 ≤ A ≤ 307 has been performed using the Coulomb and proximity potential model for deformed nuclei (CPPMDN). The alpha half-lives calculated using CPPMDN are in harmony with the values obtained by the Viola-Seaborg systematic, the universal curve of Poenaru et al., and the analytical formula of Royer. Spontaneous fission half-lives are evaluated using the new shell-effect-dependent formula proposed by Santhosh et al., and the semi-empirical formula of Xu et al. Through our study it is seen that the isotopes 300-303123 exhibit 8α chains and the isotopes 304-307123 exhibit 5α chains with half-lives in a measurable range. Clearly the isotopes of Z = 123 within the range 300 ≤ A ≤ 307 will decay through alpha emission followed by spontaneous fission and thus can be predicted as synthesized and detected in laboratory via alpha decay. Since the predictions on decay modes of isotopes of the superheavy element Z = 123 is done for the first time it is hoped that the study will open up new areas in experimental investigations.

  20. Spin density distribution in open-shell transition metal systems: A comparative post-Hartree-Fock, Density Functional Theory and quantum Monte Carlo study of the CuCl2 molecule

    CERN Document Server

    Caffarel, Michel; Scemama, Anthony; Ramírez-Solís, Alejandro

    2014-01-01

    We present a comparative study of the spatial distribution of the spin density (SD) of the ground state of CuCl2 using Density Functional Theory (DFT), quantum Monte Carlo (QMC), and post-Hartree-Fock wavefunction theory (WFT). A number of studies have shown that an accurate description of the electronic structure of the lowest-lying states of this molecule is particularly challenging due to the interplay between the strong dynamical correlation effects in the 3d shell of the copper atom and the delocalization of the 3d hole over the chlorine atoms. It is shown here that qualitatively different results for SD are obtained from these various quantum-chemical approaches. At the DFT level, the spin density distribution is directly related to the amount of Hartree-Fock exchange introduced in hybrid functionals. At the QMC level, Fixed-node Diffusion Monte Carlo (FN-DMC) results for SD are strongly dependent on the nodal structure of the trial wavefunction employed (here, Hartree-Fock or Kohn-Sham with a particula...