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Sample records for nonlinear quantum optical

  1. Quantum Computation with Nonlinear Optics

    Science.gov (United States)

    Liu, Yang; Zhang, Wen-Hong; Zhang, Cun-Lin; Long, Gui-Lu

    2008-01-01

    We propose a scheme of quantum computation with nonlinear quantum optics. Polarization states of photons are used for qubits. Photons with different frequencies represent different qubits. Single qubit rotation operation is implemented through optical elements like the Faraday polarization rotator. Photons are separated into different optical paths, or merged into a single optical path using dichromatic mirrors. The controlled-NOT gate between two qubits is implemented by the proper combination of parametric up and down conversions. This scheme has the following features: (1) No auxiliary qubits are required in the controlled-NOT gate operation; (2) No measurement is required in the course of the computation; (3) It is resource efficient and conceptually simple.

  2. Quantum Computation with Nonlinear Optics

    Institute of Scientific and Technical Information of China (English)

    LU Ke; LIU Yang; LIN Zhen-Quan; ZHANG Wen-Hong; SUN Yun-Fei; ZHANG Cun-Lin; LONG Gui-Lu

    2008-01-01

    We propose a scheme of quantum computation with nonlinear quantum optics. Polarization states of photons are used for qubits. Photons with different frequencies represent different qubits. Single qubit rotation operation is implemented through optical elements like the Faraday polarization rotator. Photons are separated into different optical paths, or merged into a single optical path using dichromatic mirrors. The controlled-NOT gate between two qubits is implemented by the proper combination of parametric up and down conversions. This scheme has the following features: (1) No auxiliary qubits are required in the controlled-NOT gate operation; (2) No measurement is required in the courseof the computation; (3) It is resource efficient and conceptually simple.

  3. Quantum nonlinear optics without photons

    Science.gov (United States)

    Stassi, Roberto; Macrı, Vincenzo; Kockum, Anton Frisk; Di Stefano, Omar; Miranowicz, Adam; Savasta, Salvatore; Nori, Franco

    2017-08-01

    Spontaneous parametric down-conversion is a well-known process in quantum nonlinear optics in which a photon incident on a nonlinear crystal spontaneously splits into two photons. Here we propose an analogous physical process where one excited atom directly transfers its excitation to a pair of spatially separated atoms with probability approaching 1. The interaction is mediated by the exchange of virtual rather than real photons. This nonlinear atomic process is coherent and reversible, so the pair of excited atoms can transfer the excitation back to the first one: the atomic analog of sum-frequency generation of light. The parameters used to investigate this process correspond to experimentally demonstrated values in ultrastrong circuit quantum electrodynamics. This approach can be extended to realize other nonlinear interatomic processes, such as four-atom mixing, and is an attractive architecture for the realization of quantum devices on a chip. We show that four-qubit mixing can efficiently implement quantum repetition codes and, thus, can be used for error-correction codes.

  4. The quantum theory of nonlinear optics

    CERN Document Server

    Drummond, Peter D

    2014-01-01

    Playing a prominent role in communications, quantum science and laser physics, quantum nonlinear optics is an increasingly important field. This book presents a self-contained treatment of field quantization and covers topics such as the canonical formalism for fields, phase-space representations and the encompassing problem of quantization of electrodynamics in linear and nonlinear media. Starting with a summary of classical nonlinear optics, it then explains in detail the calculation techniques for quantum nonlinear optical systems and their applications, quantum and classical noise sources in optical fibers and applications of nonlinear optics to quantum information science. Supplemented by end-of-chapter exercises and detailed examples of calculation techniques in different systems, this book is a valuable resource for graduate students and researchers in nonlinear optics, condensed matter physics, quantum information and atomic physics. A solid foundation in quantum mechanics and classical electrodynamic...

  5. Nonlinear optics quantum computing with circuit QED.

    Science.gov (United States)

    Adhikari, Prabin; Hafezi, Mohammad; Taylor, J M

    2013-02-08

    One approach to quantum information processing is to use photons as quantum bits and rely on linear optical elements for most operations. However, some optical nonlinearity is necessary to enable universal quantum computing. Here, we suggest a circuit-QED approach to nonlinear optics quantum computing in the microwave regime, including a deterministic two-photon phase gate. Our specific example uses a hybrid quantum system comprising a LC resonator coupled to a superconducting flux qubit to implement a nonlinear coupling. Compared to the self-Kerr nonlinearity, we find that our approach has improved tolerance to noise in the qubit while maintaining fast operation.

  6. Quantum nonlinear optics: nonlinear optics meets the quantum world (Conference Presentation)

    Science.gov (United States)

    Boyd, Robert W.

    2016-02-01

    This presentation first reviews the historical development of the field of nonlinear optics, starting from its inception in 1961. It then reviews some of its more recent developments, including especially how nonlinear optics has become a crucial tool for the developing field of quantum technologies. Fundamental quantum processes enabled by nonlinear optics, such as the creation of squeezed and entangled light states, are reviewed. We then illustrate these concepts by means of specific applications, such as the development of secure communication systems based on the quantum states of light.

  7. Quantum Information Processing using Nonlinear Optical Effects

    DEFF Research Database (Denmark)

    Andersen, Lasse Mejling

    of the converted idler depends on the other pump. This allows for temporal-mode-multiplexing. When the effects of nonlinear phase modulation (NPM) are included, the phases of the natural input and output modes are changed, reducing the separability. These effects are to some degree mediated by pre......This PhD thesis treats applications of nonlinear optical effects for quantum information processing. The two main applications are four-wave mixing in the form of Bragg scattering (BS) for quantum-state-preserving frequency conversion, and sum-frequency generation (SFG) in second-order nonlinear...... to obtain a 100 % conversion efficiency is to use multiple stages of frequency conversion, but this setup suffers from the combined effects of NPM. This problem is circumvented by using asymmetrically pumped BS, where one pump is continuous wave. For this setup, NPM is found to only lead to linear phase...

  8. Quantum and Nonlinear Optical Imaging

    Science.gov (United States)

    2007-11-02

    comment in Physical Review Letters , and more detailed versions of the theory have been written for publication. In addition, we have demonstrated...past funding cycle that was published in Physical Review Letters . This result pertains to the role of the quantum features of light in enabling the...in Physical Review Letters ) a purported theoretical demonstration of this speculation. In our work, we showed that we could reproduce this earlier

  9. Nonlinear fiber optics formerly quantum electronics

    CERN Document Server

    Agrawal, Govind

    1995-01-01

    The field of nonlinear fiber optics has grown substantially since the First Edition of Nonlinear Fiber Optics, published in 1989. Like the First Edition, this Second Edition is a comprehensive, tutorial, and up-to-date account of nonlinear optical phenomena in fiber optics. It synthesizes widely scattered research material and presents it in an accessible manner for students and researchers already engaged in or wishing to enter the field of nonlinear fiber optics. Particular attention is paid to the importance of nonlinear effects in the design of optical fiber communication systems. This is

  10. Nonlinear Quantum Optics in Artificially Structured Media

    Science.gov (United States)

    Helt, Lukas Gordon

    This thesis presents an analysis of photon pairs generated via either spontaneous parametric downconversion or spontaneous four-wave mixing in channel waveguides as well as in microring resonators side-coupled to channel waveguides. The state of photons exiting a particular device is calculated within a general Hamiltonian formalism that simplifies the link between quantum nonlinear optics experiments and classical nonlinear optics experiments. This state contains information regarding photon pair production efficiency as well as modal and spectral correlations between the two photons, characterized by a two-dimensional spectral distribution function called the biphoton wave function. In the limit of a low probability of pair production, photon pair production efficiencies are cast into forms resembling corresponding well-known classical nonlinear optical frequency conversion efficiencies, making it easy to see what plays the role of a classical "seed" field in an un-seeded (quantum) process. This also allows photon pair production efficiencies to be calculated based on the results of classical nonlinear optical experiments. It is further calculated that, unless generated photons are collected over a very narrow frequency range, their generation efficiency does not scale the same way with device length in a channel waveguide, or resonance quality factor in a microring resonator, as might be expected from the corresponding classical frequency conversion efficiency. Although calculations do not include self- or cross-phase modulation, nor two-photon absorption or free-carrier absorption, it is calculated that their neglect is justified in the low pair production probability limit. Linear (scattering) loss is also neglected, though partially addressed in the final chapter of this thesis. Biphoton wave functions are calculated explicitly, such that their shape and orientation, including approximate analytic expressions for their widths, can easily be determined. This

  11. Quantum Size- Dependent Third- Order Nonlinear Optical Susceptibility in Semiconductor Quantum Dots

    Institute of Scientific and Technical Information of China (English)

    SUN Ting; XIONG Gui-guang

    2005-01-01

    The density matrix approach has been employed to investigate the optical nonlinear polarization in a single semiconductor quantum dot(QD). Electron states are considered to be confined within a quantum dot with infinite potential barriers. It is shown, by numerical calculation, that the third-order nonlinear optical susceptibilities for a typical Si quantum dot is dependent on the quantum size of the quantum dot and the frequency of incident light.

  12. Nonlinear and quantum optics with whispering gallery resonators

    Science.gov (United States)

    Strekalov, Dmitry V.; Marquardt, Christoph; Matsko, Andrey B.; Schwefel, Harald G. L.; Leuchs, Gerd

    2016-12-01

    Optical whispering gallery modes (WGMs) derive their name from a famous acoustic phenomenon of guiding a wave by a curved boundary observed nearly a century ago. This phenomenon has a rather general nature, equally applicable to sound and all other waves. It enables resonators of unique properties attractive both in science and engineering. Very high quality factors of optical WGM resonators persisting in a wide wavelength range spanning from radio frequencies to ultraviolet light, their small mode volume, and tunable in- and out- coupling make them exceptionally efficient for nonlinear optical applications. Nonlinear optics facilitates interaction of photons with each other and with other physical systems, and is of prime importance in quantum optics. In this paper we review numerous applications of WGM resonators in nonlinear and quantum optics. We outline the current areas of interest, summarize progress, highlight difficulties, and discuss possible future development trends in these areas.

  13. Nonlinear and Quantum Optics with Whispering Gallery Resonators

    CERN Document Server

    Strekalov, Dmitry V; Matsko, Andrey B; Schwefel, Harald G L; Leuchs, Gerd

    2016-01-01

    Optical Whispering Gallery Modes (WGMs) derive their name from a famous acoustic phenomenon of guiding a wave by a curved boundary observed nearly a century ago. This phenomenon was later realized to have a rather general nature, equally applicable to sound and all other waves, but in particular also to electromagnetic waves ranging from radio frequencies to ultraviolet light. Very high quality factors of optical WGM resonators persisting in a wide wavelength range, their small mode volume, and tunable in- and out- coupling make them exceptionally efficient for nonlinear optical applications. Nonlinear optics facilitates interaction of photons with each other and with other physical systems, and is of prime importance in quantum optics. In this paper we review numerous applications of WGM resonators in nonlinear and quantum optics. We outline the current areas of interest, summarize progress, highlight difficulties, and discuss possible future development trends in these areas.

  14. Nonlinear Quantum Optical Springs and Their Nonclassical Properties

    Institute of Scientific and Technical Information of China (English)

    M.J. Faghihi; M.K. Tavassoly

    2011-01-01

    The original idea of quantum optical spring arises from the requirement of quantization of the frequency of oscillations in the Hamiltonian of harmonic oscillator. This purpose is achieved by considering a spring whose constant (and so its frequency) depends on the quantum states ofanother system. Recently, it is realized that by the assumption of frequency modulation of ω to ω √1+ μα+α the mentioned idea can be established. In the present paper, we generalize the approach of quantum optical spring with particular attention to the dependence or trequency to the intensity of radiation field that naturally observes in the nonlinear coherent states, from which we arrive at a physical system has been called by us as nonlinear quantum optical spring. Then, after the introduction of the generalized tlamiltonian of nonlinear quantum optical spring and it's solution, we will investigate the nonclassical properties of the obtained states. Specially, typical collapse and revival in the distribution functions and squeezing parameters, as particular quantum features, will be revealed.

  15. Nonlinear optics

    CERN Document Server

    Boyd, Robert W

    2013-01-01

    Nonlinear Optics is an advanced textbook for courses dealing with nonlinear optics, quantum electronics, laser physics, contemporary and quantum optics, and electrooptics. Its pedagogical emphasis is on fundamentals rather than particular, transitory applications. As a result, this textbook will have lasting appeal to a wide audience of electrical engineering, physics, and optics students, as well as those in related fields such as materials science and chemistry.Key Features* The origin of optical nonlinearities, including dependence on the polarization of light* A detailed treatment of the q

  16. Nonlinear optical signals and spectroscopy with quantum light

    CERN Document Server

    Dorfman, Konstantin E; Mukamel, Shaul

    2016-01-01

    Conventional nonlinear spectroscopy uses classical light to detect matter properties through the variation of its response with frequencies or time delays. Quantum light opens up new avenues for spectroscopy by utilizing parameters of the quantum state of light as novel control knobs and through the variation of photon statistics by coupling to matter. We present an intuitive diagrammatic approach for calculating ultrafast spectroscopy signals induced by quantum light, focusing on applications involving entangled photons with nonclassical bandwidth properties - known as "time-energy entanglement". Nonlinear optical signals induced by quantized light fields are expressed using time ordered multipoint correlation functions of superoperators. These are different from Glauber's g- functions for photon counting which use normally ordered products of ordinary operators. Entangled photon pairs are not subjected to the classical Fourier limitations on the joint temporal and spectral resolution. After a brief survey o...

  17. Nonlinear Quantum Optics in Optomechanical Nanoscale Waveguides

    CERN Document Server

    Zoubi, Hashem

    2016-01-01

    We explore the possibility of achieving a significant nonlinear phase shift among photons propagating in nanoscale waveguides exploiting interactions among photons that are mediated by vibrational modes and induced through Stimulated Brillouin Scattering (SBS). We introduce a configuration that allows slowing down the photons by several orders of magnitude via SBS involving sound waves and two pump fields. We extract the conditions for maintaining vanishing amplitude gain or loss for slowly propagating photons while keeping the influence of thermal phonons to the minimum. The nonlinear phase among two counter-propagating photons can be used to realize a deterministic phase gate.

  18. Optical Nonlinearities and Ultrafast Carrier Dynamics in Semiconductor Quantum Dots

    Energy Technology Data Exchange (ETDEWEB)

    Klimov, V.; McBranch, D.; Schwarz, C.

    1998-08-10

    Low-dimensional semiconductors have attracted great interest due to the potential for tailoring their linear and nonlinear optical properties over a wide-range. Semiconductor nanocrystals (NC's) represent a class of quasi-zero-dimensional objects or quantum dots. Due to quantum cordhement and a large surface-to-volume ratio, the linear and nonlinear optical properties, and the carrier dynamics in NC's are significantly different horn those in bulk materials. napping at surface states can lead to a fast depopulation of quantized states, accompanied by charge separation and generation of local fields which significantly modifies the nonlinear optical response in NC's. 3D carrier confinement also has a drastic effect on the energy relaxation dynamics. In strongly confined NC's, the energy-level spacing can greatly exceed typical phonon energies. This has been expected to significantly inhibit phonon-related mechanisms for energy losses, an effect referred to as a phonon bottleneck. It has been suggested recently that the phonon bottleneck in 3D-confined systems can be removed due to enhanced role of Auger-type interactions. In this paper we report femtosecond (fs) studies of ultrafast optical nonlinearities, and energy relaxation and trap ping dynamics in three types of quantum-dot systems: semiconductor NC/glass composites made by high temperature precipitation, ion-implanted NC's, and colloidal NC'S. Comparison of ultrafast data for different samples allows us to separate effects being intrinsic to quantum dots from those related to lattice imperfections and interface properties.

  19. Deterministic quantum nonlinear optics with single atoms and virtual photons

    Science.gov (United States)

    Kockum, Anton Frisk; Miranowicz, Adam; Macrı, Vincenzo; Savasta, Salvatore; Nori, Franco

    2017-06-01

    We show how analogs of a large number of well-known nonlinear-optics phenomena can be realized with one or more two-level atoms coupled to one or more resonator modes. Through higher-order processes, where virtual photons are created and annihilated, an effective deterministic coupling between two states of such a system can be created. In this way, analogs of three-wave mixing, four-wave mixing, higher-harmonic and -subharmonic generation (i.e., up- and down-conversion), multiphoton absorption, parametric amplification, Raman and hyper-Raman scattering, the Kerr effect, and other nonlinear processes can be realized. In contrast to most conventional implementations of nonlinear optics, these analogs can reach unit efficiency, only use a minimal number of photons (they do not require any strong external drive), and do not require more than two atomic levels. The strength of the effective coupling in our proposed setups becomes weaker the more intermediate transition steps are needed. However, given the recent experimental progress in ultrastrong light-matter coupling and improvement of coherence times for engineered quantum systems, especially in the field of circuit quantum electrodynamics, we estimate that many of these nonlinear-optics analogs can be realized with currently available technology.

  20. Optimization of optical nonlinearities in quantum cascade lasers

    Science.gov (United States)

    Bai, Jing

    Nonlinearities in quantum cascade lasers (QCL's) have wide applications in wavelength tunability and ultra-short pulse generation. In this thesis, optical nonlinearities in InGaAs/AlInAs-based mid-infrared (MIR) QCL's with quadruple resonant levels are investigated. Design optimization for the second-harmonic generation (SHG) of the device is presented. Performance characteristics associated with the third-order nonlinearities are also analyzed. The design optimization for SHG efficiency is obtained utilizing techniques from supersymmetric quantum mechanics (SUSYQM) with both material-dependent effective mass and band nonparabolicity. Current flow and power output of the structure are analyzed by self-consistently solving rate equations for the carriers and photons. Nonunity pumping efficiency from one period of the QCL to the next is taken into account by including all relevant electron-electron (e-e) and longitudinal (LO) phonon scattering mechanisms between the injector/collector and active regions. Two-photon absorption processes are analyzed for the resonant cascading triple levels designed for enhancing SHG. Both sequential and simultaneous two-photon absorption processes are included in the rate-equation model. The current output characteristics for both the original and optimized structures are analyzed and compared. Stronger resonant tunneling in the optimized structure is manifested by enhanced negative differential resistance. Current-dependent linear optical output power is derived based on the steady-state photon populations in the active region. The second-harmonic (SH) power is derived from the Maxwell equations with the phase mismatch included. Due to stronger coupling between lasing levels, the optimized structure has both higher linear and nonlinear output powers. Phase mismatch effects are significant for both structures leading to a substantial reduction of the linear-to-nonlinear conversion efficiency. The optimized structure can be fabricated

  1. Linear and nonlinear optical susceptibilities in a laterally coupled quantum-dot–quantum-ring system

    Energy Technology Data Exchange (ETDEWEB)

    Zeng, Zaiping; Garoufalis, Christos S.; Baskoutas, Sotirios, E-mail: bask@upatras.gr

    2014-07-18

    Linear and nonlinear optical susceptibilities in a laterally coupled quantum-dot–quantum-ring system have been theoretically studied. In general, we find that the structure parameters of the coupled system significantly affect the optical susceptibilities. The enhancement of the coupling effects between the dot and ring is found to increase considerably the optical susceptibilities and redshift drastically the transition energies. Comparing to the linear susceptibility, the nonlinear optical susceptibility is found to be more sensitive to the variation of the structure parameters. A comprehensive analysis of the electron probability density movement with respect to the modification of the structure parameters is provided, which offers a unique perspective of the ground-state localization. - Highlights: • Optical susceptibilities in a quantum-dot–quantum-ring system are studied. • The structure parameters significantly affect the optical susceptibilities. • The enhancement of the coupling effects increases the optical susceptibilities. • The nonlinear susceptibility is more sensitive to the change in structure parameters. • A comprehensive analysis of the electron probability density movement is provided.

  2. Size Dependent Optical Nonlinearity and Optical Limiting Properties of Water Soluble CdSe Quantum Dots

    Directory of Open Access Journals (Sweden)

    Anju K. Augustine

    2014-01-01

    Full Text Available We present third-order optical nonlinear absorption in CdSe quantum dots (QDs with particle sizes in the range of 4.16–5.25 nm which has been evaluated by the Z-scan technique. At an excitation irradiance of 0.54 GW/cm2 the CdSe QDs exhibit reverse saturation indicating a clear nonlinear behavior. Nonlinearity increases with particle size in CdSe QDs within the range of our investigations which in turn depends on the optical band gap. The optical limiting threshold of the QDs varies from 0.35 GW/cm2 to 0.57 GW/cm2 which makes CdSe QDs a promising candidate for reverse-saturable absorption based devices at high laser intensities such as optical limiters.

  3. Nonlinear optical switching and optical limiting in colloidal CdSe quantum dots investigated by nanosecond Z-scan measurement

    Science.gov (United States)

    Valligatla, Sreeramulu; Haldar, Krishna Kanta; Patra, Amitava; Desai, Narayana Rao

    2016-10-01

    The semiconductor nanocrystals are found to be promising class of third order nonlinear optical materials because of quantum confinement effects. Here, we highlight the nonlinear optical switching and optical limiting of cadmium selenide (CdSe) quantum dots (QDs) using nanosecond Z-scan measurement. The intensity dependent nonlinear absorption and nonlinear refraction of CdSe QDs were investigated by applying the Z-scan technique with 532 nm, nanosecond laser pulses. At lower intensities, the nonlinear process is dominated by saturable absorption (SA) and it is changed to reverse saturable absorption (RSA) at higher intensities. The SA behaviour is attributed to the ground state bleaching and the RSA is ascribed to free carrier absorption (FCA) of CdSe QDs. The nonlinear optical switching behaviour and reverse saturable absorption makes CdSe QDs are good candidate for all-optical device and optical limiting applications.

  4. Hybrid quantum systems for enhanced nonlinear optical susceptibilities

    CERN Document Server

    Sullivan, Dennis; Kuzyk, Mark G

    2016-01-01

    Significant effort has been expended in the search for materials with ultra-fast nonlinear-optical susceptibilities, but most fall far below the fundamental limits. This work applies a theoretical materials development program that has identified a promising new hybrid made of a nanorod and a molecule. This system uses the electrostatic dipole moment of the molecule to break the symmetry of the metallic nanostructure that shifts the energy spectrum to make it optimal for a nonlinear-optical response near the fundamental limit. The structural parameters are varied to determine the ideal configuration, providing guidelines for making the best structures.

  5. Numerical simulation of linear and nonlinear quantum optics as a design tool for free-space quantum communications and quantum imaging

    Science.gov (United States)

    Meyers, Ronald E.; Deacon, Keith S.; Rosen, D.

    2002-12-01

    A new quantum optics tool for simulating quantum probability density functions resulting from the linear and nonlinear interaction of photons with atoms and with other photons is developed and presented. It can be used to design and simulate quantum optics experiments used in quantum communications, quantum computing, and quantum imaging. Examples of a photon interacting with linears systems of mirrors and beamsplitters are simulated. Nonlinear simulations of the interaction of three photons resulting in photon momentum entanglement is presented. The wavefunction is expanded in Fock states. Fock states cannot be represented by classical modeling and therefore, the results of our modeling can in general represent phenomena in both the linear and nonlinear cases which cannot be modeled by classical linear optics. The modeling presented here is more general than the classical linear optics. Models of atmospheric turbulence and their simulations are presented and demonstrate the potential for first principles physics quantum optics simulations through turbulence in realistic environments.

  6. Nonlinear carrier dynamics in a quantum dash optical amplifier

    DEFF Research Database (Denmark)

    Hansen, Per Lunnemann; Ek, Sara; Yvind, Kresten

    2012-01-01

    Results of experimental pump-probe spectroscopy of a quantum dash optical amplifier biased at transparency are presented. Using strong pump pulses we observe a competition between free carrier absorption and two-photon induced stimulated emission that can have drastic effects on the transmission ...

  7. Control of optical bistability and third-order nonlinearity via tunneling induced quantum interference in triangular quantum dot molecules

    Energy Technology Data Exchange (ETDEWEB)

    Tian, Si-Cong, E-mail: tiansicong@ciomp.ac.cn; Tong, Cun-Zhu, E-mail: tongcz@ciomp.ac.cn; Zhang, Jin-Long; Shan, Xiao-Nan; Fu, Xi-Hong; Zeng, Yu-Gang; Qin, Li; Ning, Yong-Qiang [State Key laboratory of Luminescence and Applications, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033 (China); Wan, Ren-Gang [School of Physics and Information Technology, Shaanxi Normal University, Xi’an 710062 (China)

    2015-06-15

    The optical bistability of a triangular quantum dot molecules embedded inside a unidirectional ring cavity is studied. The type, the threshold and the hysteresis loop of the optical bistability curves can be modified by the tunneling parameters, as well as the probe laser field. The linear and nonlinear susceptibilities of the medium are also studied to interpret the corresponding results. The physical interpretation is that the tunneling can induce the quantum interference, which modifies the linear and the nonlinear response of the medium. As a consequence, the characteristics of the optical bistability are changed. The scheme proposed here can be utilized for optimizing and controlling the optical switching process.

  8. Quantum nonlinear optics with polar J-aggregates in microcavities

    CERN Document Server

    Herrera, Felipe; Pachon, Leonardo A; Saikin, Semion K; Aspuru-Guzik, Alán

    2014-01-01

    We show that an ensemble of organic dye molecules with permanent electric dipole moments embedded in a microcavity can lead to strong optical nonlinearities at the single photon level. The strong long-range electrostatic interaction between chromophores due to their permanent dipoles introduces the desired nonlinearity of the light-matter coupling in the microcavity. We obtain the absorption spectra of a weak probe field under the influence of strong exciton-photon coupling with the cavity field. Using realistic parameters, we demonstrate that a single cavity photon can significantly modify the absorptive and dispersive response of the medium to a probe photon at a different frequency. Finally, we show that the system is in the regime of cavity-induced transparency with a broad transparency window for dye dimers. We illustrate our findings using pseudoisocyanine chloride (PIC) J-aggregates in currently-available optical microcavities.

  9. The nonlinear optical rectification of a confined exciton in a quantum dot

    Energy Technology Data Exchange (ETDEWEB)

    Xie Wenfang, E-mail: xiewf@gzhu.edu.c [School of Physics and Electronic Engineering, Guangzhou University, Guangzhou 510006 (China)

    2011-05-15

    An exciton in a disc-like quantum dot (QD) with the parabolic confinement, under applied electric field, is studied within the framework of the effective-mass approximation. The nonlinear optical rectification between the ground and the first-excited states has been examined through the computed energies and wave functions in details for the excitons. The results show that the optical rectification susceptibility obtained in a disc-like QD reach the magnitude of 10{sup -2} m/V, which is 3-4 orders of magnitude higher than in one-dimensional QDs. It is found that the second-order nonlinear optical properties of exciton states in a QD are strongly affected by the confinement strength and the electric field. - Research highlights: {yields} The magnitude of the nonlinear optical rectification of the excitons confined in a disc-like quantum dot may reach 10{sup -2} m/V. It is much higher than that of the other low-dimensional semiconductors, e.g., quantum wells, and one-dimensional semiparabolic quantum dots. {yields} The nonlinear optical rectification of the excitons confined in a disc-like quantum dot is strongly dependent on the confinement frequency. In order to obtain the larger optical rectification coefficients in quantum dots, we can change the confinement frequency. {yields} The calculated results also reveal that an applied electric field has a great influence on the nonlinear optical rectification susceptibility. In order to obtain the larger optical rectification coefficients in quantum dots we can induce the electric field.

  10. Nonlinear carrier dynamics in a quantum dash optical amplifier

    DEFF Research Database (Denmark)

    Hansen, Per Lunnemann; Ek, Sara; Yvind, Kresten;

    2012-01-01

    Results of experimental pump-probe spectroscopy of a quantum dash optical amplifier biased at transparency are presented. Using strong pump pulses we observe a competition between free carrier absorption and two-photon induced stimulated emission that can have drastic effects on the transmission...... dynamics. Thus, both enhancement as well as suppression of the transmission can be observed even when the amplifier is biased at transparency. A simple theoretical model taking into account two-photon absorption and free carrier absorption is presented that shows good agreement with the measurements....

  11. Electric field effect on the second-order nonlinear optical properties in semiparabolic quantum wells

    Science.gov (United States)

    Yuan, Jian-Hui; Chen, Ni; Zhang, Yan; Mo, Hua; Zhang, Zhi-Hai

    2016-03-01

    Electric field effect on the second-order nonlinear optical properties in semiparabolic quantum wells are studied theoretically. Both the second-harmonic generation susceptibility and nonlinear optical rectification depend dramatically on the direction and the strength of the electric field. Numerical results show that both the second-harmonic generation susceptibility and nonlinear optical rectification are always weakened as the electric field increases where the direction of the electric field is along the growth direction of the quantum wells, which is in contrast to the conventional case. However, the second-harmonic generation susceptibility is weakened, but the nonlinear optical rectification is strengthened as the electric field increases where the direction of the electric field is against the growth direction of the quantum wells. Also it is the blue (or red) shift of the resonance that is induced by increasing of the electric field when the direction of the electric field is along (or against) the growth direction of the quantum wells. Finally, the resonant peak and its corresponding to the resonant energy are also taken into account.

  12. Nonlinear optics

    CERN Document Server

    Bloembergen, Nicolaas

    1996-01-01

    Nicolaas Bloembergen, recipient of the Nobel Prize for Physics (1981), wrote Nonlinear Optics in 1964, when the field of nonlinear optics was only three years old. The available literature has since grown by at least three orders of magnitude.The vitality of Nonlinear Optics is evident from the still-growing number of scientists and engineers engaged in the study of new nonlinear phenomena and in the development of new nonlinear devices in the field of opto-electronics. This monograph should be helpful in providing a historical introduction and a general background of basic ideas both for expe

  13. Nonlinear optical systems

    CERN Document Server

    Lugiato, Luigi; Brambilla, Massimo

    2015-01-01

    Guiding graduate students and researchers through the complex world of laser physics and nonlinear optics, this book provides an in-depth exploration of the dynamics of lasers and other relevant optical systems, under the umbrella of a unitary spatio-temporal vision. Adopting a balanced approach, the book covers traditional as well as special topics in laser physics, quantum electronics and nonlinear optics, treating them from the viewpoint of nonlinear dynamical systems. These include laser emission, frequency generation, solitons, optically bistable systems, pulsations and chaos and optical pattern formation. It also provides a coherent and up-to-date treatment of the hierarchy of nonlinear optical models and of the rich variety of phenomena they describe, helping readers to understand the limits of validity of each model and the connections among the phenomena. It is ideal for graduate students and researchers in nonlinear optics, quantum electronics, laser physics and photonics.

  14. Optical Nonlinear Properties of CdSeS/ZnS Core/Shell Quantum Dots

    Institute of Scientific and Technical Information of China (English)

    WU Feng; TIAN Wei; MA Li-Na; CHEN Wen-Ju; ZHANG Gui-Lan; ZHAO Guo-Feng; CAO Shi-Dong; XIE Wei

    2008-01-01

    @@ The optical nonlinear properties of CdSeS/ZnS quantum dots (QDs) are investigated by Z-scan technique using fundamental harmonic generation (1064nm) of mode-locked Nd:YAG laser for the first time. The experimental results show that two photon absorptions (TPA) occur at input intensity up to 12.5 GW/cm2. CdSeS/ZnS QDs have an average TPA cross section of 13710GM and large nonlinear refractive index on order of 10-7 esu. The large optical nonlinearities perhaps allow the CdSeS/ZnS QDs to be one kind of candidate material for bioimaging and fluorescence label, optical limiting and all-optical switching.

  15. Nonlinear optics response of semiconductor quantum wells under high magnetic fields

    Energy Technology Data Exchange (ETDEWEB)

    Chemla, D.S.

    1993-07-01

    Recent investigations on the nonlinear optical response of semiconductor quantum wells in a strong perpendicular magnetic field, H, are reviewed. After some introductory material the evolution of the linear optical properties of GaAs QW`s as a function of H is discussed; an examination is made of how the magneto-excitons (MX) extrapolate continuously between quasi-2D QW excitons (X) when H = 0, and pairs of Landau levels (LL) when H {yields} {infinity}. Next, femtosecond time resolved investigations of their nonlinear optical response are presented; the evolution of MX-MX interactions with increasing H is stressed. Finally, how, as the dimensionality is reduced by application of H, the number of scattering channels is limited and relaxation of electron-hole pairs is affected. How nonlinear optical spectroscopy can be exploited to access the relaxation of angular momentum within magneto-excitons is also discussed.

  16. Electronic absorption spectra and nonlinear optical properties of CO2 molecular aggregates: A quantum chemical study

    Indian Academy of Sciences (India)

    Tarun K Mandal; Sudipta Dutta; Swapan K Pati

    2009-09-01

    We have investigated the structural aspects of several carbon dioxide molecular aggregates and their spectroscopic and nonlinear optical properties within the quantum chemical theory framework. We find that, although the single carbon dioxide molecule prefers to be in a linear geometry, the puckering of angles occur in oligomers because of the intermolecular interactions. The resulting dipole moments reflect in the electronic excitation spectra of the molecular assemblies. The observation of significant nonlinear optical properties suggests the potential application of the dense carbon dioxide phases in opto-electronic devices.

  17. The preparation of the nonlinear optical quantum dots in organic polymer composite

    Science.gov (United States)

    Huang, Guochang; Yu, Dabin; Zhang, Jinhua; Zhao, Minghui; Zhao, Dapeng; Pan, Maosen

    2016-11-01

    Quantum dots (QDs) is some material which particle size is between 1 to 10 nanometers. Because of the unique nonlinear optical properties, QDs has been widely applied in optical, electrical, magnetic, biological fields etc. Though the size of the nanoscale is bringing the QDs a series of characteristic advantages, it has also brought some problems for further application, such as QDs are easily degenerative according to their small size. However, The preparation of quantum dots with special polymer composite film can avoid this phenomenon, This means that the composite is usually with inert matrix can be realized for further application.

  18. Quantum-enhanced tunable second-order optical nonlinearity in bilayer graphene.

    Science.gov (United States)

    Wu, Sanfeng; Mao, Li; Jones, Aaron M; Yao, Wang; Zhang, Chuanwei; Xu, Xiaodong

    2012-04-11

    Second order optical nonlinear processes involve the coherent mixing of two electromagnetic waves to generate a new optical frequency, which plays a central role in a variety of applications, such as ultrafast laser systems, rectifiers, modulators, and optical imaging. However, progress is limited in the mid-infrared (MIR) region due to the lack of suitable nonlinear materials. It is desirable to develop a robust system with a strong, electrically tunable second order optical nonlinearity. Here, we demonstrate theoretically that AB-stacked bilayer graphene (BLG) can exhibit a giant and tunable second order nonlinear susceptibility χ((2)) once an in-plane electric field is applied. χ((2)) can be electrically tuned from 0 to ~10(5) pm/V, 3 orders of magnitude larger than the widely used nonlinear crystal AgGaSe(2). We show that the unusually large χ((2)) arise from two different quantum enhanced two-photon processes thanks to the unique electronic spectrum of BLG. The tunable electronic bandgap of BLG adds additional tunability on the resonance of χ((2)), which corresponds to a tunable wavelength ranging from ~2.6 to ~3.1 μm for the up-converted photon. Combined with the high electron mobility and optical transparency of the atomically thin BLG, our scheme suggests a new regime of nonlinear photonics based on BLG. © 2012 American Chemical Society

  19. Nanofiber Fabry-Perot microresonator for non-linear optics and cavity quantum electrodynamics

    CERN Document Server

    Wuttke, C; Brückner, S; Rothhardt, M; Rauschenbeutel, A

    2012-01-01

    We experimentally realize a Fabry-Perot-type optical microresonator near the cesium D2 line wavelength based on a tapered optical fiber, equipped with two fiber Bragg gratings which enclose a sub-wavelength diameter waist. Owing to the very low taper losses, the finesse of the resonator reaches F = 86 while the on-resonance transmission is T = 11 %. The characteristics of our resonator fulfill the requirements of non-linear optics and cavity quantum electrodynamics in the strong coupling regime. In combination with its demonstrated ease of use and its advantageous mode geometry, it thus opens a realm of applications.

  20. Nanofiber Fabry-Perot microresonator for nonlinear optics and cavity quantum electrodynamics.

    Science.gov (United States)

    Wuttke, C; Becker, M; Brückner, S; Rothhardt, M; Rauschenbeutel, A

    2012-06-01

    We experimentally realize a Fabry-Perot-type optical microresonator near the cesium D2 line wavelength based on a tapered optical fiber, equipped with two fiber Bragg gratings that enclose a subwavelength diameter waist. Owing to the very low taper losses, the finesse of the resonator reaches F=86 while the on-resonance transmission is T=11%. The characteristics of our resonator fulfill the requirements of nonlinear optics and cavity quantum electrodynamics in the strong coupling regime. These characteristics, combined with the demonstrated ease of use and advantageous mode geometry, open a realm of applications.

  1. Nonlinear optical properties of free standing films of PbS quantum dots in the nonresonant femtosecond regime

    Science.gov (United States)

    Kurian, Pushpa Ann; Vijayan, C.; Nag, Amit; Goswami, Debabrata

    2013-01-01

    Devices based on optical technology for high speed communication networks require materials with large nonlinear optical response in the ultrafast regime. Nonlinear optical materials have also attracted wide attention as potential candidates for the protection of optical sensors and eyes while handling lasers. Optical limiters have a constant transmittance at low input influence and a decrease in transmittance at higher fluences and are based on a variety of mechanisms such as nonlinear refraction, nonlinear scattering, multiphoton absorption and free carrier absorption. As we go from bulk to nanosized materials especially in the strong quantum confinement regime where radius of the nanoparticle is less than the bulk exciton Bohr radius, the optical nonlinearity is enhanced due to quantum confinement effect. This paper is on the ultrafast nonresonant nonlinearity in free standing films of PbS quantum dots stabilized in a synthetic glue matrix by a simple chemical route which provides flexibility of processing in a variety of physical forms. Optical absorption spectrum shows significant blue shift from the bulk absorption onset indicating strong quantum confinement. PbS quantumdots of mean size 3.3nm are characterized by X-ray diffraction and transmission electron microscopy. The mechanism of nonlinear absorption giving rise to optical limiting is probed using open z-scan technique with laser pulses of 150 fs pulse duration at 780 nm and the results are presented in the nonresonant femtosecond regime. Irradiance dependence on nonlinear absorption are discussed. PMID:24143059

  2. Nonlinear optical properties of free standing films of PbS quantum dots in the nonresonant femtosecond regime.

    Science.gov (United States)

    Kurian, Pushpa Ann; Vijayan, C; Nag, Amit; Goswami, Debabrata

    2007-09-17

    Devices based on optical technology for high speed communication networks require materials with large nonlinear optical response in the ultrafast regime. Nonlinear optical materials have also attracted wide attention as potential candidates for the protection of optical sensors and eyes while handling lasers. Optical limiters have a constant transmittance at low input influence and a decrease in transmittance at higher fluences and are based on a variety of mechanisms such as nonlinear refraction, nonlinear scattering, multiphoton absorption and free carrier absorption. As we go from bulk to nanosized materials especially in the strong quantum confinement regime where radius of the nanoparticle is less than the bulk exciton Bohr radius, the optical nonlinearity is enhanced due to quantum confinement effect. This paper is on the ultrafast nonresonant nonlinearity in free standing films of PbS quantum dots stabilized in a synthetic glue matrix by a simple chemical route which provides flexibility of processing in a variety of physical forms. Optical absorption spectrum shows significant blue shift from the bulk absorption onset indicating strong quantum confinement. PbS quantumdots of mean size 3.3nm are characterized by X-ray diffraction and transmission electron microscopy. The mechanism of nonlinear absorption giving rise to optical limiting is probed using open z-scan technique with laser pulses of 150 fs pulse duration at 780 nm and the results are presented in the nonresonant femtosecond regime. Irradiance dependence on nonlinear absorption are discussed.

  3. Zeolite Y Films as Ideal Platform for Evaluation of Third-Order Nonlinear Optical Quantum Dots

    Directory of Open Access Journals (Sweden)

    Hyun Sung Kim

    2016-01-01

    Full Text Available Zeolites are ideal host material for generation and stabilization of regular ultrasmall quantum dots (QDs array with the size below 1.5 nm. Quantum dots (QDs with high density and extinction absorption coefficient have been expected to give high level of third-order nonlinear optical (3rd-NLO and to have great potential applications in optoelectronics. In this paper, we carried out a systematic elucidation of the third-order nonlinear optical response of various types of QDs including PbSe, PbS, CdSe, CdS, ZnSe, ZnS, Ag2Se, and Ag2S by manipulation of QDs into zeolites Y pores. In this respect, we could demonstrate that the zeolite offers an ideal platform for capability comparison 3rd-NLO response of various types of QDs with high sensitivities.

  4. Analysis on nonlinear optical properties of Cd (Zn) Se quantum dots synthesized using three different stabilizing agents

    Science.gov (United States)

    J, Joy Sebastian Prakash; G, Vinitha; Ramachandran, Murugesan; Rajamanickam, Karunanithi

    2017-10-01

    Three different stabilizing agents, namely, L-cysteine, Thioglycolic acid and cysteamine hydrochloride were used to synthesize Cd(Zn)Se quantum dots (QDs). It was characterized using UV-vis spectroscopy, x-ray diffraction (XRD) and transmission electron microscopy (TEM). The non-linear optical properties (non-linear absorption and non-linear refraction) of synthesized Cd(Zn)Se quantum dots were studied with z-scan technique using diode pumped continuous wavelaser system at a wavelength of 532 nm. Our (organic) synthesized quantum dots showed optical properties similar to the inorganic materials reported elsewhere.

  5. General solution to nonlinear optical quantum graphs using Dalgarno-Lewis summation techniques

    CERN Document Server

    Lytel, Rick; Kuzyk, Mark G

    2016-01-01

    We develop an algorithm to apply the Dalgarno-Lewis (DL) perturbation theory to quantum graphs with multiple, connected edges. We use it to calculate the nonlinear optical hyperpolarizability tensors for graphs and show that it replicates the sum over states computations, but executes ten to fifty times faster. DL requires only knowledge of the ground state of the graph, eliminating the requirement to determine all possible degeneracies of a complex network. The algorithm is general and may be applied to any quantum graph.

  6. High-order optical nonlinearities in nanocomposite films dispersed with semiconductor quantum dots at high concentrations

    Science.gov (United States)

    Tomita, Yasuo; Matsushima, Shun-suke; Yamagami, Ryu-ichi; Jinzenji, Taka-aki; Sakuma, Shohei; Liu, Xiangming; Izuishi, Takuya; Shen, Qing

    2017-06-01

    We describe the nonlinear optical properties of inorganic-organic nanocomposite films in which semiconductor CdSe quantum dots as high as 6.8 vol.% are dispersed. Open/closed Z-scan measurements, degenerate multi-wave mixing and femtosecond pump-probe/transient grating measurements are conducted. It is shown that the observed fifth-order optical nonlinearity has the cascaded third-order contribution that becomes prominent at high concentrations of CdSe QDs. It is also shown that there are picosecond-scale intensity-dependent and nanosecond-scale intensity-independent decay components in absorptive and refractive nonlinearities. The former is caused by the Auger process, while the latter comes from the electron-hole recombination process.

  7. Optical nonlinearity for few-photon pulses on a quantum dot-pillar cavity device

    CERN Document Server

    Loo, Vivien; Gazzano, Olivier; Lemaitre, Aristide; Sagnes, Isabelle; Krebs, Olivier; Voisin, Paul; Senellart, Pascale; Lanco, Loïc

    2012-01-01

    Giant optical nonlinearity is observed under both continuous-wave and pulsed excitation in a deterministically-coupled quantum dot-micropillar system, in a pronounced strong-coupling regime. Using absolute reflectivity measurements we determine the critical intracavity photon number as well as the input and output coupling efficiencies of the device. Thanks to a near-unity input-coupling efficiency, we demonstrate a record nonlinearity threshold of only 8 incident photons per pulse. The output-coupling efficiency is found to strongly influence this nonlinearity threshold. We show how the fundamental limit of single-photon nonlinearity can be attained in realistic devices, which would provide an effective interaction between two coincident single photons.

  8. Nonlinear optical response in a zincblende GaN cylindrical quantum dot with donor impurity center

    Energy Technology Data Exchange (ETDEWEB)

    Hoyos, Jaime H. [Departamento de Ciencias Básicas, Universidad de Medellín, Cra. 87 No. 30-65, Medellín (Colombia); Correa, J.D., E-mail: jcorrea@udem.edu.co [Departamento de Ciencias Básicas, Universidad de Medellín, Cra. 87 No. 30-65, Medellín (Colombia); Mora-Ramos, M.E. [Centro de Investigación en Ciencias, Instituto de Investigación en Ciencias Básicas y Aplicadas, Universidad Autónoma del Estado de Morelos, Av. Universidad 1001, CP 62209 Cuernavaca, Morelos (Mexico); Duque, C.A. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia)

    2016-03-01

    We calculate the nonlinear optical absorption coefficient of a cylindrical zincblende GaN-based quantum dot. For this purpose, we consider Coulomb interactions between electrons and an impurity ionized donor atom. The electron-donor-impurity spectrum and the associated quantum states are calculated using the effective mass approximation with a parabolic potential energy model describing both the radial and axial electron confinement. We also include the effects of the hydrostatic pressure and external electrostatic fields. The energy spectrum is obtained through an expansion of the eigenstates as a linear combination of Gaussian-type functions which reduces the computational effort since all the matrix elements are obtained analytically. Therefore, the numerical problem is reduced to the direct diagonalization of the Hamiltonian. The obtained energies are used in the evaluation of the dielectric susceptibility and the nonlinear optical absorption coefficient within a modified two-level approach in a rotating wave approximation. This quantity is investigated as a function of the quantum dot dimensions, the impurity position, the external electric field intensity and the hydrostatic pressure. The results of this research could be important in the design and fabrication of zincblende GaN-quantum-dot-based electro-optical devices.

  9. Optical nonlinearities of iron doped zinc sulphide quantum dots

    Science.gov (United States)

    Cinumon, K. V.; Prasanth, S.; Raj, D. Rithesh; Vineeshkumar, T. V.; Pillai, V. P. Mahadevan; Sudarsanakumar, C.

    2017-05-01

    Polyethylene glycol (PEG) capped pure and Fe doped ZnS nanoparticles were successfully synthesized by chemical precipitation method. Cubic zinc blende phase of the samples was confirmed from X-ray diffraction. The average grain size was found to be in the range of 2-3 nm and was confirmed with TEM. The undoped and doped ZnS samples show blue emission with emission wavelength at 360 nm. A rapid luminescence quenching with increasing dopant concentration was observed. The nonlinear absorption coefficients of the doped and undoped samples were calculated using Z-scan technique.

  10. Handbook of nonlinear optical crystals

    CERN Document Server

    Dmitriev, Valentin G; Nikogosyan, David N

    1991-01-01

    This Handbook of Nonlinear Optical Crystals provides a complete description of the properties and applications of nonlinear crystals In addition, it presents the most important equations for calculating the main parameters of nonlinear frequency converters This comprehensive reference work will be of great value to all scientists and engineers working in nonlinear optics, quantum electronics and laser physics

  11. Effects of graphene quantum dots on linear and nonlinear optical behavior of malignant ovarian cells

    Science.gov (United States)

    Mohajer, Salman; Ara, Mohammad Hossein Majles; Serahatjoo, Leila

    2016-07-01

    We investigate linear and nonlinear optical properties of standard human ovarian cancer cells (cell line: A2780cp) in vitro. Cells were treated by graphene quantum dots (GQDs) with two special concentrations. Nontoxicity of GQDs was examined in standard biological viability tests. Cancerous cells were fixed on a glass slide; then, interaction of light with biofilms was studied in linear and nonlinear regimes. Absorption spectra of untreated biofilms and biofilms with two different concentrations of GQDs was studied by UV-visible spectrophotometer. Optical behavior of biofilms in a linear regime of intensity (with low-intensity laser exposure) was reported using a simple optical setup. After that, we compared the attenuation of light in biofilm of cancerous cells with and without GQDs. Nonlinear behavior of these biofilms was investigated by a Z-scan setup using a continued wave He-Ne laser. Results showed that GQDs decreased the extinction coefficient and changed the sign and exact value of the nonlinear refractive index of malignant ovarian cells noticeably. The nonlinear refractive index of studied cells with no GQDs treatment was in the order of 10-8 (cm2/w) with a positive sign. This quantity changed to the same order of magnitude with a negative sign after GQDs treatment. Thus, GQDs can be used for cancer diagnosis under laser irradiation.

  12. Linear and nonlinear optical absorption coefficients of two-electron spherical quantum dot with parabolic potential

    Science.gov (United States)

    Çakır, Bekir; Yakar, Yusuf; Özmen, Ayhan

    2015-02-01

    Linear and nonlinear absorption coefficients of two-electron spherical quantum dot (QD) with parabolic potential are investigated in this paper. Wave functions and energy eigenvalues of the 1s2, 1s1p, 1s1d and 1s1f electronic states have been computed by using an optimization approach, which is a combination of Quantum Genetic Algorithm (QGA) and Hartree-Fock Roothaan (HFR) method. It is found that the strength of S→P transition is stronger than P→D and D→F transitions. Also the peak positions and amplitudes of the absorption coefficients are sensitive to the electron spin. It should be noted that the peak positions and amplitudes of absorption coefficients are strongly dependent on the parabolic potential. Additionally, dot radius, impurity charge, incident optical intensity and relaxation time have a great influence on the linear and nonlinear absorption coefficients.

  13. Linear and nonlinear optical absorption coefficients of two-electron spherical quantum dot with parabolic potential

    Energy Technology Data Exchange (ETDEWEB)

    Çakır, Bekir, E-mail: bcakir@selcuk.edu.tr [Physics Department, Faculty of Science, Selcuk University, Campus 42075, Konya (Turkey); Yakar, Yusuf, E-mail: yuyakar@yahoo.com [Physics Department, Faculty of Arts and Science, Aksaray University, Campus 68100, Aksaray (Turkey); Özmen, Ayhan [Physics Department, Faculty of Science, Selcuk University, Campus 42075, Konya (Turkey)

    2015-02-01

    Linear and nonlinear absorption coefficients of two-electron spherical quantum dot (QD) with parabolic potential are investigated in this paper. Wave functions and energy eigenvalues of the 1s{sup 2}, 1s1p, 1s1d and 1s1f electronic states have been computed by using an optimization approach, which is a combination of Quantum Genetic Algorithm (QGA) and Hartree–Fock Roothaan (HFR) method. It is found that the strength of S→P transition is stronger than P→D and D→F transitions. Also the peak positions and amplitudes of the absorption coefficients are sensitive to the electron spin. It should be noted that the peak positions and amplitudes of absorption coefficients are strongly dependent on the parabolic potential. Additionally, dot radius, impurity charge, incident optical intensity and relaxation time have a great influence on the linear and nonlinear absorption coefficients.

  14. Strongly driven nonlinear quantum optics in microring resonators

    CERN Document Server

    Vernon, Z

    2015-01-01

    We present a detailed analysis of strongly driven spontaneous four-wave mixing in a lossy integrated microring resonator side-coupled to a channel waveguide. A nonperturbative, analytic solution within the undepleted pump approximation is developed for a cw pump input of arbitrary intensity. In the strongly driven regime self- and cross-phase modulation, as well as multi-pair generation, lead to a rich variety of power-dependent effects; the results are markedly different than in the low power limit. The photon pair generation rate, single photon spectrum, and joint spectral intensity (JSI) distribution are calculated. Splitting of the generated single photon spectrum into a doublet structure associated with both pump detuning and cross-phase modulation is predicted, as well as substantial narrowing of the generated signal and idler bandwidths associated with the onset of optical parametric oscillation at intermediate powers. Both the correlated and uncorrelated contributions to the JSI are calculated, and fo...

  15. Quantum optical waveform conversion

    CERN Document Server

    Kielpinski, D; Wiseman, HM

    2010-01-01

    Currently proposed architectures for long-distance quantum communication rely on networks of quantum processors connected by optical communications channels [1,2]. The key resource for such networks is the entanglement of matter-based quantum systems with quantum optical fields for information transmission. The optical interaction bandwidth of these material systems is a tiny fraction of that available for optical communication, and the temporal shape of the quantum optical output pulse is often poorly suited for long-distance transmission. Here we demonstrate that nonlinear mixing of a quantum light pulse with a spectrally tailored classical field can compress the quantum pulse by more than a factor of 100 and flexibly reshape its temporal waveform, while preserving all quantum properties, including entanglement. Waveform conversion can be used with heralded arrays of quantum light emitters to enable quantum communication at the full data rate of optical telecommunications.

  16. Effects of Electron-Phonon Interaction on Linear and Nonlinear Optical Absorption in Cylindrical Quantum Wires

    Institute of Scientific and Technical Information of China (English)

    YU You-Bin

    2008-01-01

    The electron-phonon interaction influences on linear and nonlinear optical absorption in cylindrical quantum wires (CQW) with an infinite confining potential are investigated. The optical absorption coefficients are obtained by using the compact-density-matrix approach and iterative method, and the numerical results are presented for GaAs CQW. The results show that the electron-phonon interaction makes a distinct influence on optical absorption in CQW. The electron-phonon interaction on the wave functions of electron dominates the values of absorption coefficients and the correction of the electron-phonon effect on the energies of the electron makes the absorption peaks blue shift and become wider. Moreover, the electron-phonon interaction influence on optical absorption with an infinite confining potential is different from that with a finite confining potential.

  17. Impurity-related nonlinear optical properties in delta-doped quantum rings: Electric field effects

    Energy Technology Data Exchange (ETDEWEB)

    Restrepo, R.L., E-mail: rrestre@gmail.com [Escuela de Ingeniería de Antioquia-EIA, Medellín (Colombia); Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia); Morales, A.L. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia); Martínez-Orozco, J.C. [Unidad Académica de Física, Universidad Autónoma de Zacatecas, CP 98060, Zacatecas (Mexico); Baghramyan, H.M.; Barseghyan, M.G. [Department of Solid State Physics, Yerevan State University, Al. Manookian 1, 0025 Yerevan (Armenia); Mora-Ramos, M.E. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia); Facultad de Ciencias, Universidad Autónoma del Estado de Morelos, Ave. Universidad 1001, CP 62209, Cuernavaca, Morelos (Mexico); Duque, C.A. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia)

    2014-11-15

    Using a variational procedure within the effective mass approximation, we have calculated the donor impurity binding energy for the ground (1s-like) and the excited (2p{sub z}-like) states as well as the impurity-related nonlinear optical absorption and relative changes in the refraction index in a GaAs single quantum ring with axial n-type delta-doping. The delta-like potential along the z-direction is an approximate model analytically described using a Lorentzian function with two parameters. Additionally we consider the application of an electric field along the z-direction. It is found that the changes in the geometry of the quantum ring, the change in the 2D impurity density of the delta-like doping, and different values of the electric field lead to a shifting of the resonant peaks of the optical responses spectrum.

  18. Nonlinear optical properties of near-infrared region Ag2S quantum dots pumped by nanosecond laser pulses

    Directory of Open Access Journals (Sweden)

    Li-wei Liu

    2015-08-01

    Full Text Available This study investigates near-infrared region Ag2S quantum dots (QDs and their nonlinear optical response under 532 nm nanosecond laser pulses. Our experimental result shows that nonlinear transmission is reduced from 0.084 to 0.04. The observed narrowing behavior of the output pulse width shows superior optical limiting. We discuss the physical mechanisms responsible for the nonlinear optical response of the QDs. The average size of the nanocrystals was 5.5 nm. Our results suggest the possibility of using these Ag2S QDs for photoelectric, biosensor, optical ranging, and self-adaptive technologies.

  19. Linear and Nonlinear Optical Absorptions of a Hydrogenic Donor in a Quantum Dot Under a Magnetic Field

    Institute of Scientific and Technical Information of China (English)

    XIE Wen-Fang

    2009-01-01

    The linear and nonlinear optical properties of a hydrogenic donor in a disc-like parabolic quantum dot in the presence of an external magnetic field are studied. The calculations were performed within the effective mass approximation, using the matrix diagonalization method and the compact density-matrix approach. The linear and nonlinear optical absorption coefficients between the ground (L = 0) and the first excited state (L = 1) have been examined based on the computed energies and wave functions. We find that the linear, nonlinear third-order, and total optical absorption coefficients are strongly affected by the confinement strength of QDs, the external magnetic field, and the incident optical intensity.

  20. Focus issue introduction: nonlinear optics 2013.

    Science.gov (United States)

    Dadap, Jerry I; Karlsson, Magnus; Panoiu, Nicolae C

    2013-12-16

    Nonlinear Optics has continued to develop over the last few years at an extremely fast pace, with significant advances being reported in nonlinear optical metamaterials, optical signal processing, quantum optics, nonlinear optics at subwavelength scale, and biophotonics. These exciting new developments have generated significant potential for a broad spectrum of technological applications in which nonlinear-optical processes play a central role.

  1. Optimizing optical nonlinearities in GaInAs/AlInAs quantum cascade lasers

    Directory of Open Access Journals (Sweden)

    Gajić Aleksandra D.

    2014-01-01

    Full Text Available Regardless of the huge advances made in the design and fabrication of mid-infrared and terahertz quantum cascade lasers, success in accessing the ~3-4 mm region of the electromagnetic spectrum has remained limited. This fact has brought about the need to exploit resonant intersubband transitions as powerful nonlinear oscillators, consequently enabling the occurrence of large nonlinear optical susceptibilities as a means of reaching desired wavelengths. In this work, we present a computational model developed for the optimization of second-order optical nonlinearities in In0.53Ga0.47As/Al0.48In0.52As quantum cascade laser structures based on the implementation of the Genetic algorithm. The carrier transport and the power output of the structure were calculated by self-consistent solutions to the system of rate equations for carriers and photons. Both stimulated and simultaneous double-photon absorption processes occurring between the second harmonic generation-relevant levels are incorporated into rate equations and the material-dependent effective mass and band non-parabolicity are taken into account, as well. The developed method is quite general and can be applied to any higher order effect which requires the inclusion of the photon density equation. [Projekat Ministarstva nauke Republike Srbije, br. III 45010

  2. Quantum nonlinear optics with single photons enabled by strongly interacting atoms

    DEFF Research Database (Denmark)

    Peyronel, Thibault; Firstenberg, Ofer; Liang, Qi Yu

    2012-01-01

    The realization of strong nonlinear interactions between individual light quanta (photons) is a long-standing goal in optical science and engineering, being of both fundamental and technological significance. In conventional optical materials, the nonlinearity at light powers corresponding...

  3. Nonlinear optical effects and Hong-Ou-Mandel interference in cavity quantum electrodynamics

    Science.gov (United States)

    Mirza, Imran M.; van Enk, Steven J.

    Pure quantum interference among single photons is one of the key ingredients to perform linear optics quantum computation (LOQC). The Hong-Ou-Mandel interference (HOMI) [C. K. Hong, Z. Y. Ou and L. Mandel, Phys. Rev. Lett. 59, (18), 2044-2046 (1987)] i.e. complete destructive interference between two identical and indistinguishable photons simultaneously entering input ports of a 50/50 beam splitter, is a well-known example in this context. In this talk, I'll present our theoretical study of HOMI in a coupled Jaynes-Cummings array. In particular and by applying quantum jump/trajectory formalism, I'll focus on how partial quantum interference between two photons survive both non-linearities produced by two-level emitter and spectral filtering due to optical cavities in our coupled cavity array setup [Imran M. Mirza and Steven J. van Enk, Opt. Comm. 343, 172-177 (2015)]. Along with LOQC, this work is crucial from the perspective of exploiting coupled cavity arrays to store single photons reliably (without altering their temporal and spectral traits) [Imran M. Mirza, Steven J. van Enk and Jeff Kimble, JOSA B, 10, 2640-2649, (2013)].

  4. Spin–orbit interaction effect on nonlinear optical rectification of quantum wire in the presence of electric and magnetic fields

    Energy Technology Data Exchange (ETDEWEB)

    Kumar, Manoj [Department of Physics and Astrophysics, University of Delhi, Delhi 110007 (India); Lahon, Siddhartha, E-mail: sid.lahon@gmail.com [Department of Physics and Astrophysics, University of Delhi, Delhi 110007 (India); Department of Physics, Kirori Mal College, University of Delhi, Delhi 110007 (India); Jha, Pradip Kumar [Department of Physics and Astrophysics, University of Delhi, Delhi 110007 (India); Department of Physics, DDU College, University of Delhi, Delhi 110007 (India); Gumber, Sukirti; Mohan, Man [Department of Physics and Astrophysics, University of Delhi, Delhi 110007 (India)

    2014-04-01

    Here we have investigated the influence of external electric field and magnetic field on the nonlinear optical rectification of a parabolic confinement wire in the presence of Rashba spin–orbit interaction. We have used density matrix formulation for obtaining optical properties within the effective mass approximation. The results are presented as a function of quantum wire radius, electric field, magnetic field, Rashba spin–orbit interaction strength and photon energy. Our results indicate an increase of electric field gives the red-shift of the peak positions of nonlinear optical rectification. The role of confinement strength and spin–orbit interaction strength as control parameters on this nonlinear property have been demonstrated.

  5. First Example of Nonlinear Optical Materials Based on Nanoconjugates of Sandwich Phthalocyanines with Quantum Dots.

    Science.gov (United States)

    Oluwole, David O; Yagodin, Alexey V; Mkhize, Nhlakanipho C; Sekhosana, Kutloano E; Martynov, Alexander G; Gorbunova, Yulia G; Tsivadze, Aslan Yu; Nyokong, Tebello

    2017-02-24

    We report original, selective, and efficient approaches to novel nonlinear optical (NLO) materials, namely homoleptic double- and triple-decker europium(III) complexes 2 and 3 with the A3 B-type phthalocyanine ligand (2,3-bis[2'-(2''-hydroxyethoxy)ethoxy]-9,10,16,17,23,24-hexa-n-butoxyphthalocyanine 1) bearing two anchoring diethyleneglycol chains terminated with OH groups. Their covalently linked nanoconjugates with mercaptosuccinic acid-capped ternary CdSeTe/CdTeS/ZnSeS quantum dots are prepared in the presence of an ethyl(dimethylaminopropyl)carbodiimide activating agent. Optical limiting (OL) properties of the obtained low-symmetry complexes and their conjugates with quantum dots (QDs) are measured for the first time by the open-aperture Z-scan technique (532 nm laser and pulse rate of 10 ns). For comparison, symmetrical double- and triple-decker Eu(III) octa-n-butoxyphthalocyaninates 5 and 6 and their mixtures with trioctylphosphine oxide-capped QDs are also synthesized and studied. It is revealed that both lowering of molecular symmetry and expansion of the π-electron system upon moving from double- to triple-decker complexes significantly improves the OL characteristics, making the low-symmetry triple-decker complex 3 the most efficient optical limiter in the studied family of sandwich complexes, affording 50 % lowering of light transmittance below 0.5 J cm(-2) input fluence. Conjugation (both covalent and noncovalent) with QDs affords further enhancement of the OL properties of both double- and triple-decker complexes. Altogether, the obtained results contribute to the development of novel nonlinear optical materials for future nanoelectronic and optical device applications. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

  6. Remote Atmospheric Nonlinear Optical Magnetometry

    Science.gov (United States)

    2014-04-28

    Boyd , Nonlinear Optics (Elsevier, Burlington, MA, 2008). [13] M. Scully and S. Zubairy, Quantum Optics (Cambridge U. Press, Cambridge, UK, 1997...Naval Research Laboratory Washington, DC 20375-5320 NRL/MR/6703--14-9548 Remote Atmospheric Nonlinear Optical Magnetometry PhilliP SPrangle...b. ABSTRACT c. THIS PAGE 18. NUMBER OF PAGES 17. LIMITATION OF ABSTRACT Remote Atmospheric Nonlinear Optical Magnetometry Phillip Sprangle, Luke

  7. Quantum well nonlinear microcavities

    Science.gov (United States)

    Oudar, J. L.; Kuszelewicz, R.; Sfez, B.; Pellat, D.; Azoulay, R.

    We report on recent progress in reducing the power threshold of all-optical bistable quantum well vertical microcavities. Significant improvements are achieved through an increase of the cavity finesse, together with a reduction of the device active layer thickness. A critical intensity of 5 μW/μm 2 has been observed on a microcavity of finesse 250, with a nonlinear medium of only 18 GaAs quantum wells of 10 nm thickness. Further improvements of the Bragg mirror quality resulted in a finesse of 700 and a power-lifetime product of 15 fJ/μm 2. Microresonator pixellation allows to obtain 2-dimensional arrays. A thermally-induced alloy-mixing technique is described, which produced a 110 meV carrier confinement energy, together with a refractive index change of -.012, averaged over the 2.6 μm nonlinear medium thickness. The resulting electrical and optical confinement is shown to improve the nonlinear characteristics, by limiting lateral carrier diffusion and light diffraction.

  8. Nonlinear optical characterization of colloidal solutions containing dye and Ag2S quantum dot associates

    Science.gov (United States)

    Boltaev, G. S.; Sobirov, B.; Reyimbaev, S.; Sherniyozov, H.; Usmanov, T.; Smirnov, M. S.; Ovchinnikov, O. V.; Grevtseva, I. G.; Kondratenko, T. S.; Shihaliev, H. S.; Ganeev, R. A.

    2016-12-01

    We analyzed the nonlinear absorption and refraction in the dyes and silver sulfide quantum dot (QD) associates. The nonlinear refractive indices, nonlinear absorption coefficients, and third-order nonlinear susceptibilities of the Ag2S QDs associated with various dyes (xanthenes, thiazines, carbocyanines, quinolines) were measured. The influence of dyes nonlinearities on the whole pattern of the z-scans of colloidal QD solutions, as well as the application of different molar fractions of dyes and intensities of probe radiation (40 ps, 1064 nm and 532 nm), were analyzed and discussed in the contest of the influence of various nonlinear absorption processes.

  9. Dark-gray soliton transformations: possibility to study microscopic quantum phenomena by nonlinear optical methods

    Science.gov (United States)

    Hernández-Tenorio, C.; Serkin, V. N.; Belyaeva, T. L.; Peña-Moreno, R.; Morales-Lara, L.

    2015-01-01

    The nonlinear Schrödinger equation (NLSE) model with an external harmonic potential is one of the most important in modern science. This model makes it possible to analyze a variety of nonlinear phenomena, in nonlinear optics and laser physics, biophysics and in the theory of Bose-Einstein condensation of atoms. It is shown that the main specific feature of the dynamics of dark GP matter wave solitons in a parabolic trap is the formation of solitons with dynamically changing form-factors producing the periodic variation in the modulation depth (the degree of "blackness") of dark solitons. In general, the period of dark soliton oscillations in trapping potential depends on the specific conditions of the experiment and does not coincide with the oscillation period of a linear quantum-mechanical oscillator. In the case of an immobile pedestal in the trap, the oscillation period of the black soliton considerably increases because of the periodic transformation of the black soliton to the gray one and vice versa. Surprisingly, that if the dark soliton is superimposed on the base pedestal oscillating in the trap and displaced from the trap center, the oscillation period of the dark soliton coincides with the period of oscillations of the linear harmonic oscillator, while the dynamics of the dark soliton is similar to that of a classical particle obeying the Newton mechanics laws.

  10. Linear and nonlinear intersubband optical properties in a triangular quantum ring

    Energy Technology Data Exchange (ETDEWEB)

    Nasri, Djillali [Faculté des Sciences Appliquées, Département de Génie Electrique, Université Ibn-Khaldoun de Tiaret, Zaaroura BP No.78, Tiaret 14000 (Algeria); Laboratoire de Microphysique et de Nanophysique (LaMiN), Ecole Nationale Polytechnique d’Oran, BP 1523 EL M’Naouer, Oran 31000 (Algeria); Bettahar, N [Faculté des Sciences de la matière, Département de Physique, Université Ibn-Khaldoun de Tiaret, Zaaroura, BP No.78, Tiaret 14000 (Algeria)

    2015-12-01

    Using the effective mass approximation, within the plane wave expansion, the linear and nonlinear coefficients absorption and the refractive index changes relative to the intersubband transitions in the conduction band of an Al{sub x}Ga{sub 1−x}As/ GaAs/Al{sub x}Ga{sub 1−x}As triangular quantum ring for an x-polarization and an y-polarization of the incident light are calculated. It is found that the transition energy between the ground state and the first two excited states and their related optical matrix are strongly influenced by the length of the side of the inner triangle, leading to a red-shift and blue-shift of the resonant peaks of the intersubband optical absorption, for an x-polarized light absorption and an y-polarized light absorption respectively. Our results are qualitatively similar to those of a triangular quantum wire in the presence of an intense laser field in recent literature.

  11. Electronic states and the resonant optical non-linearity of exciton in a narrow band InSb quantum dot

    Energy Technology Data Exchange (ETDEWEB)

    Narayanan, M. [Department of Physics, Yadava College Govindarajan Campus, Thiruppalai, Madurai-625 014 (India); John Peter, A., E-mail: a.john.peter@gmail.com [Center for Environmental Studies/Green Energy Center, Department of Environmental Science and Engineering, College of Engineering, Kyung Hee University, Seocheon-dong 1, Giheung-gu, Yongin-Si, Gyeonggi-Do, 446-701 (Korea, Republic of); Yoo, Chang Kyoo [Center for Environmental Studies/Green Energy Center, Department of Environmental Science and Engineering, College of Engineering, Kyung Hee University, Seocheon-dong 1, Giheung-gu, Yongin-Si, Gyeonggi-Do, 446-701 (Korea, Republic of)

    2012-02-01

    Binding energy, interband emission energy and the non-linear optical properties of exciton in an InSb/InGa{sub x}Sb{sub 1-x} quantum dot are computed as functions of dot radius and the Ga content. Optical properties are obtained using the compact density matrix approach. The dependence of non-linear optical processes on the dot sizes is investigated for different Ga concentrations. The linear, third order non-linear optical absorption coefficients, susceptibility values and the refractive index changes of the exciton are calculated for different concentrations of gallium content. It is found that gallium concentration has great influence on the optical properties of InSb/InGa{sub x}Sb{sub 1-x} dots.

  12. Linear and nonlinear optical properties of multilayered spherical quantum dots: Effects of geometrical size, hydrogenic impurity, hydrostatic pressure and temperature

    Energy Technology Data Exchange (ETDEWEB)

    Karimi, M.J. [Department of Physics, College of Sciences, Shiraz University of Technology, Shiraz 71555-313 (Iran, Islamic Republic of); Rezaei, G., E-mail: grezaei2001@gmail.com [Department of Physics, College of Sciences, Yasouj University, Yasouj 75914-353 (Iran, Islamic Republic of); Nazari, M. [Department of Physics, College of Sciences, Shiraz University of Technology, Shiraz 71555-313 (Iran, Islamic Republic of); Department of Physics, College of Sciences, Yasouj University, Yasouj 75914-353 (Iran, Islamic Republic of)

    2014-01-15

    Based on the effective mass and parabolic one band approximations, simultaneous effects of the geometrical size, hydrogenic impurity, hydrostatic pressure, and temperature on the intersubband optical absorption coefficients and refractive index changes in multilayered spherical quantum dots are studied. Energy eigenvalues and eigenvectors are calculated using the fourth-order Runge–Kutta method and optical properties are obtained using the compact density matrix approach. The results indicate that the hydrogenic impurity, hydrostatic pressure, temperature and geometrical parameters such as the well and barrier widths have a great influence on the linear, the third-order nonlinear and the total optical absorption coefficients and refractive index changes. -- Highlights: • Hydrogenic impurity effects on the optical properties of a MSQD are investigated. • Hydrostatic pressure and temperature effects are also studied. • Hydrogenic impurity has a great influence on the linear and nonlinear ACs and RICs. • Hydrostatic pressure and temperature change the linear and nonlinear ACs and RICs.

  13. Enhancement of surface plasmon resonances on the nonlinear optical properties in a GaAs quantum dot

    Science.gov (United States)

    Jiang, Xiancong; Guo, Kangxian; Liu, Guanghui; Yang, Tao; Yang, Yanlian

    2017-05-01

    In this paper, the nonlinear optical properties of a metallic nanoparticle (MNP)-semiconductor quantum dot (SQD) hybrid nanosystem with the hybrid exciton effect have been studied. Considering the influence of quantum-size effect to the dielectric function of MNP, the quantum corrected dielectric function was applied to our calculation. By using the compact-density-matrix method, the interaction between MNP and SQD has been studied theoretically. The results show that the surface plasmon resonances (SPRs) of MNP enhance indeed the nonlinear optical properties of SQD. Further more, the enhancement depends on two factors: (a) the center-to-center 7distance between MNP and SQD; (b) the radius ratio between MNP and SQD.

  14. UV Nano-Lights: Nonlinear Quantum Dot-Plasmon Coupling

    Science.gov (United States)

    2014-08-01

    method is also applicable to bare nanoparticles in polar solvents. 15. SUBJECT TERMS Quantum Dots, Nonlinear Optical Materials , Energy...TERMS Quantum Dots, Nonlinear Optical Materials , Energy Conservation, Up-conversion 16. SECURITY CLASSIFICATION OF: 17. LIMITATION OF ABSTRACT

  15. Nonlinear optical rectification in laterally-coupled quantum well wires with applied electric field

    Science.gov (United States)

    Liu, Guanghui; Guo, Kangxian; Zhang, Zhongmin; Hassanbadi, Hassan; Lu, Liangliang

    2017-03-01

    Nonlinear optical rectification coefficient χ0(2) in laterally-coupled AlxGa1-xAs/GaAs quantum well wires with an applied electric field is theoretically investigated using the effective mass approximation as well as the numerical energy levels and wavefunctions of electrons. We find that χ0(2) is greatly influenced by the electric field as well as both the distance and the radius of the coupled system. A blue shift of χ0(2) with increasing electric field is exhibited while a red shift followed by a blue shift with increasing distance or radius is exhibited. A nonmonotonic behavior can be found in the resonant peak values of χ0(2) along with the increase of the electric field, the distance or the radius. One or two of the following physical mechanisms: the increased localization of the ground and first-excited states, the reduced coupling and the reduced quantum confinement effect are applied to elucidate the results above. Our results play a potential role in infrared photodetectors based on the coupled system.

  16. Lectures on light nonlinear and quantum optics using the density matrix

    CERN Document Server

    Rand, Stephen C.

    2016-01-01

    This book bridges the gap between introductory quantum mechanics and the research front of modern optics and scientific fields that make use of light. While suitable as a reference for the specialist in quantum optics, it also targets non-specialists from other disciplines who need to understand light and its uses in research. It introduces a single analytic tool, the density matrix, to analyze complex optical phenomena encountered in traditional as well as cross-disciplinary research. It moves swiftly in a tight sequence from elementary to sophisticated topics in quantum optics, including optical tweezers, laser cooling, coherent population transfer, optical magnetism, electromagnetically induced transparency, squeezed light, and cavity quantum electrodynamics. A systematic approach starts with the simplest systems—stationary two-level atoms—then introduces atomic motion, adds more energy levels, and moves on to discuss first-, second-, and third-order coherence effects that are the basis for analyzing n...

  17. Optical nonlinear response function with linear and diagonal quadratic electron-vibration coupling in mixed quantum-classical systems.

    Science.gov (United States)

    Toutounji, Mohamad

    2005-03-22

    While an optical linear response function of linearly and quadratically coupled mixed quantum-classical condensed-phase systems was derived by Toutounji [J. Chem. Phys. 121, 2228 (2004)], the corresponding analytical optical line shape is derived. The respective nonlinear correlation functions are also derived. Model calculations involving photon-echo, pump-probe, and hole-burning signals of model systems with both linear and quadratic coupling are provided. Hole-burning formula of Hayes-Small is compared to that of Mukamel in mixed quantum-classical systems.

  18. Linear and nonlinear intraband optical properties of ZnO quantum dots embedded in SiO2 matrix

    Directory of Open Access Journals (Sweden)

    Deepti Maikhuri

    2012-03-01

    Full Text Available In this work we investigate some optical properties of semiconductor ZnO spherical quantum dot embedded in an amorphous SiO2 dielectric matrix. Using the framework of effective mass approximation, we have studied intraband S-P, and P-D transitions in a singly charged spherical ZnO quantum dot. The optical properties are investigated in terms of the linear and nonlinear photoabsorption coefficient, the change in refractive index, and the third order nonlinear susceptibility and oscillator strengths. Using the parabolic confinement potential of electron in the dot these parameters are studied with the variation of the dot size, and the energy and intensity of incident radiation. The photoionization cross sections are also obtained for the different dot radii from the initial ground state of the dot. It is found that dot size, confinement potential, and incident radiation intensity affects intraband optical properties of the dot significantly.

  19. Applications of nonlinear fiber optics

    CERN Document Server

    Agrawal, Govind

    2008-01-01

    * The only book describing applications of nonlinear fiber optics * Two new chapters on the latest developments: highly nonlinear fibers and quantum applications* Coverage of biomedical applications* Problems provided at the end of each chapterThe development of new highly nonlinear fibers - referred to as microstructured fibers, holey fibers and photonic crystal fibers - is the next generation technology for all-optical signal processing and biomedical applications. This new edition has been thoroughly updated to incorporate these key technology developments.The bo

  20. Quantum optics

    DEFF Research Database (Denmark)

    Andersen, Ulrik Lund

    2013-01-01

    Further sensitivity improvements are required before advanced optical interferometers will be able to measure gravitational waves. A team has now shown that introducing quantum squeezing of light may help to detect these elusive waves.......Further sensitivity improvements are required before advanced optical interferometers will be able to measure gravitational waves. A team has now shown that introducing quantum squeezing of light may help to detect these elusive waves....

  1. Quantum optics

    DEFF Research Database (Denmark)

    Andersen, Ulrik Lund

    2013-01-01

    Further sensitivity improvements are required before advanced optical interferometers will be able to measure gravitational waves. A team has now shown that introducing quantum squeezing of light may help to detect these elusive waves.......Further sensitivity improvements are required before advanced optical interferometers will be able to measure gravitational waves. A team has now shown that introducing quantum squeezing of light may help to detect these elusive waves....

  2. Electron-related linear and nonlinear optical responses in vertically coupled triangular quantum dots

    Energy Technology Data Exchange (ETDEWEB)

    Martínez-Orozco, J.C. [Unidad Académica de Física. Universidad Autónoma de Zacatecas, Calzada Solidaridad esquina con Paseo la Bufa S/N, C.P. 98060. Zacatecas, Zac. (Mexico); Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia); Mora-Ramos, M.E. [Facultad de Ciencias, Universidad Autónoma del Estado de Morelos, Ave. Universidad 1001, CP 62209, Cuernavaca, Morelos (Mexico); Duque, C.A., E-mail: cduque@fisica.udea.edu.co [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia)

    2014-11-01

    The conduction band states of GaAs-based vertically coupled double triangular quantum dots in two dimensions are investigated within the effective mass and parabolic approximation, using a diagonalization procedure to solve the corresponding Schrödinger-like equation. The effect of an externally applied static electric field is included in the calculation, and the variation of the lowest confined energy levels as a result of the change of the field strength is reported for different geometrical setups. The linear and nonlinear optical absorptions and the relative change of the refractive index, associated with the energy transition between the ground and the first excited state in the system, are studied as a function of the incident light frequency for distinct configurations of inter-dot distance and electric field intensities. The blueshift of the resonant absorption peaks is detected as a consequence of the increment in the field intensity, whereas the opposite effect is obtained from the increase of inter-dot vertical distance. It is also shown that for large enough values of the electric field there is a quenching of the optical absorption due to field-induced change of symmetry of the first excited state wavefunction, in the case of triangular dots of equal shape and size.

  3. Introductory Quantum Optics

    Science.gov (United States)

    Gerry, Christopher; Knight, Peter

    2004-10-01

    1. Introduction; 2. Field quantization; 3. Coherent states; 4. Emission and absorption of radiation by atoms; 5. Quantum coherence functions; 6. Beam splitters and interferometers; 7. Nonclassical light; 8. Dissipative interactions and decoherence; 9. Optical test of quantum mechanics; 10. Experiments in cavity QED and with trapped ions; 11. Applications of entanglement: Heisenberg-limited interferometry and quantum information processing; Appendix A. The density operator, entangled states, the Schmidt decomposition, and the von Neumann entropy; Appendix B. Quantum measurement theory in a (very small) nutshell; Appendix C. Derivation of the effective Hamiltonian for dispersive (far off-resonant) interactions; Appendix D. Nonlinear optics and spontaneous parametric down-conversion.

  4. Hydrostatic pressure and temperature effects on nonlinear optical rectification in a lens shape InAs/GaAs quantum dot

    Energy Technology Data Exchange (ETDEWEB)

    Bouzaieene, L., E-mail: lotfi.bouzaiene@fsm.rnu.tn [Laboratoire de Micro-optoelectronique et Nanostructures, Departement de Physique, Faculte des Sciences de Monastir, Universite de Monastir (Tunisia); Ben Mahrsia, R.; Baira, M.; Sfaxi, L.; Maaref, H. [Laboratoire de Micro-optoelectronique et Nanostructures, Departement de Physique, Faculte des Sciences de Monastir, Universite de Monastir (Tunisia)

    2013-03-15

    We have performed theoretical calculation of the nonlinear optical rectification in a lens shape InAs/GaAs quantum dot (0D). The combined effects of hydrostatic pressure and temperature on the nonlinear optical rectification in lens-shaped InAs QDs are studied under the compact density matrix formalism and the effective mass approximation. From our calculation, it is found that the subband energies and optical rectification susceptibility are quite sensitive to the applied hydrostatic pressure and temperature. The results show that the resonant peak of the optical rectification can be red-shifted or blue-shifted and their intensity also varied by external probes such as hydrostatic pressure and temperature. In addition, the oscillator strength is strongly affected by these parameters. - Highlights: Black-Right-Pointing-Pointer Theoretical calculation of the nonlinear optical rectification in a lens shape InAs/GaAs quantum dot was performed. Black-Right-Pointing-Pointer Optical rectification susceptibility is quite sensitive to the applied hydrostatic pressure and temperature. Black-Right-Pointing-Pointer The oscillator strength is strongly affected by the applied hydrostatic pressure and temperature.

  5. Study of optical non-linear properties of a constant total effective length multiple quantum wells system

    Energy Technology Data Exchange (ETDEWEB)

    Solaimani, M.; Morteza, Izadifard [Faculty of Physics, Shahrood University of technology, Shahrood (Iran, Islamic Republic of); Arabshahi, H., E-mail: arabshahi@um.ac.ir [Department of Physics, Ferdowsi University of Mashhad, Mashhad (Iran, Islamic Republic of); Physics Department, Payame Noor University, P.O. Box 19395-3697, Tehran (Iran, Islamic Republic of); Reza, Sarkardehi Mohammad [Physics Department, Al-Zahra University, Vanak, Tehran (Iran, Islamic Republic of)

    2013-02-15

    In this work, we have studied the effect of the number of the wells, in a multiple quantum wells structure with constant total effective length, on the optical properties of multiple quantum wells like the absorption coefficient and the refractive index by means of compact density matrix approach. GaAs/Al{sub x}Ga{sub (1-x)}As multiple quantum wells systems was selected as an example. Besides, the effect of varying number of wells on the subband energies, wave functions, number of bound states, and the Fermi energy have been also investigated. Our calculation revealed that the number of wells in a multiple quantum well is a criterion with which we can control the amount of nonlinearity. This study showed that for the third order refractive index change there is two regimes of variations and the critical well number was six. In our calculations, we have used the same wells and barrier thicknesses to construct the multiple quantum wells system. - Highlights: Black-Right-Pointing-Pointer OptiOptical Non-Linear. Black-Right-Pointing-Pointer Total Effective Length. Black-Right-Pointing-Pointer Multiple Quantum Wells System - genetic algorithm Black-Right-Pointing-Pointer Schroedinger equation solution. Black-Right-Pointing-Pointer Nanostructure.

  6. Effects of electromagnetic fields on the nonlinear optical properties of asymmetric double quantum well under intense laser field

    Science.gov (United States)

    Yesilgul, U.; Sari, H.; Ungan, F.; Martínez-Orozco, J. C.; Restrepo, R. L.; Mora-Ramos, M. E.; Duque, C. A.; Sökmen, I.

    2017-03-01

    In this study, the effects of electric and magnetic fields on the optical rectification and second and third harmonic generation in asymmetric double quantum well under the intense non-resonant laser field is theoretically investigated. We calculate the optical rectification and second and third harmonic generation within the compact density-matrix approach. The theoretical findings show that the influence of electric, magnetic, and intense laser fields leads to significant changes in the coefficients of nonlinear optical rectification, second and third harmonic generation.

  7. Advances in nonlinear optics

    CERN Document Server

    Chen, Xianfeng; Zeng, Heping; Guo, Qi; She, Weilong

    2015-01-01

    This book presents an overview of the state of the art of nonlinear optics from weak light nonlinear optics, ultrafast nonlinear optics to electro-optical theory and applications. Topics range from the fundamental studies of the interaction between matter and radiation to the development of devices, components, and systems of tremendous commercial interest for widespread applications in optical telecommunications, medicine, and biotechnology.

  8. Lossless synthesis of graphene nanosheets decorated with tiny cadmium sulfide quantum dots with excellent nonlinear optical properties.

    Science.gov (United States)

    Feng, Miao; Sun, Ruiqing; Zhan, Hongbing; Chen, Yu

    2010-02-19

    The implantation and growth of metal nanoparticles on graphene nanosheets (GNS) leads directly to severe damage to the regular structure of the graphene sheets, which disrupts the extended pi conjugation, resulting in an impaired device performance. In this paper, we describe a facile approach for achieving the lossless formation of graphene composite decorated with tiny cadmium sulfide quantum dots (QDs) with excellent nonlinear optical properties by using benzyl mercaptan (BM) as the interlinker. The mercapto substituent of BM binds to the CdS QDs during their nucleation and growth process, and then the phenyl comes into contact with the GNS via the pi-pi stacking interaction. Using this strategy, CdS QDs with an average diameter of 3 nm are uniformly dispersed over the surface of graphene, and the resulting QD-graphene composite exhibits excellent optical limiting properties, mainly contributed by nonlinear scattering and nonlinear absorption, upon both 532 and 1064 nm excitations, in the nanosecond laser pulse regime.

  9. Nonlinear optical spectra having characteristics of Fano interferences in coherently coupled lowest exciton biexciton states in semiconductor quantum dots

    Directory of Open Access Journals (Sweden)

    Hideki Gotoh

    2014-10-01

    Full Text Available Optical nonlinear effects are examined using a two-color micro-photoluminescence (micro-PL method in a coherently coupled exciton-biexciton system in a single quantum dot (QD. PL and photoluminescence excitation spectroscopy (PLE are employed to measure the absorption spectra of the exciton and biexciton states. PLE for Stokes and anti-Stokes PL enables us to clarify the nonlinear optical absorption properties in the lowest exciton and biexciton states. The nonlinear absorption spectra for excitons exhibit asymmetric shapes with peak and dip structures, and provide a distinct contrast to the symmetric dip structures of conventional nonlinear spectra. Theoretical analyses with a density matrix method indicate that the nonlinear spectra are caused not by a simple coherent interaction between the exciton and biexciton states but by coupling effects among exciton, biexciton and continuum states. These results indicate that Fano quantum interference effects appear in exciton-biexciton systems at QDs and offer important insights into their physics.

  10. Quantum Optics

    CERN Document Server

    Garrison, J C

    2008-01-01

    Quantum optics, i.e. the interaction of individual photons with matter, began with the discoveries of Planck and Einstein, but in recent years it has expanded beyond pure physics to become an important driving force for technological innovation. This book serves the broader readership growing out of this development by starting with an elementary description of the underlying physics and then building up a more advanced treatment. The reader is led from the quantum theory of thesimple harmonic oscillator to the application of entangled states to quantum information processing. An equally impor

  11. Analysis of optical parity gates of generating Bell state for quantum information and secure quantum communication via weak cross-Kerr nonlinearity under decoherence effect

    Science.gov (United States)

    Heo, Jino; Hong, Chang-Ho; Yang, Hyung-Jin; Hong, Jong-Phil; Choi, Seong-Gon

    2017-04-01

    We demonstrate the advantages of an optical parity gate using weak cross-Kerr nonlinearities (XKNLs), quantum bus (qubus) beams, and photon number resolving (PNR) measurement through our analysis, utilizing a master equation under the decoherence effect (occurred the dephasing and photon loss). To generate Bell states, parity gates based on quantum non-demolition measurement using XKNL are extensively employed in quantum information processing. When designing a parity gate via XKNL, the parity gate can be diversely constructed according to the measurement strategies. In practice, the interactions of XKNLs in optical fiber are inevitable under the decoherence effect. Thus, by our analysis of the decoherence effect, we show that the designed parity gate employing homodyne measurement would not be expected to provide reliable quantum operation. Furthermore, compared with a parity gate using a displacement operator and PNR measurement, we conclude there is experimental benefit from implementation of a parity gate via qubus beams and PNR measurement under the decoherence effect.

  12. 4-wave mixing for phase-matching free nonlinear optics in quantum cascade structures : LDRD 08-0346 final report.

    Energy Technology Data Exchange (ETDEWEB)

    Chow, Weng Wah; Wanke, Michael Clement; Allen, Dan G.; Yang, Zhenshan; Waldmueller, Ines

    2010-10-01

    Optical nonlinearities and quantum coherences have the potential to enable efficient, high-temperature generation of coherent THz radiation. This LDRD proposal involves the exploration of the underlying physics using intersubband transitions in a quantum cascade structure. Success in the device physics aspect will give Sandia the state-of-the-art technology for high-temperature THz quantum cascade lasers. These lasers are useful for imaging and spectroscopy in medicine and national defense. Success may have other far-reaching consequences. Results from the in-depth study of coherences, dephasing and dynamics will eventually impact the fields of quantum computing, optical communication and cryptology, especially if we are successful in demonstrating entangled photons or slow light. An even farther reaching development is if we can show that the QC nanostructure, with its discrete atom-like intersubband resonances, can replace the atom in quantum optics experiments. Having such an 'artificial atom' will greatly improve flexibility and preciseness in experiments, thereby enhancing the discovery of new physics. This is because we will no longer be constrained by what natural can provide. Rather, one will be able to tailor transition energies and optical matrix elements to enhance the physics of interest. This report summarizes a 3-year LDRD program at Sandia National Laboratories exploring optical nonlinearities in intersubband devices. Experimental and theoretical investigations were made to develop a fundamental understanding of light-matter interaction in a semiconductor system and to explore how this understanding can be used to develop mid-IR to THz emitters and nonclassical light sources.

  13. Impurity-related linear and nonlinear optical response in quantum-well wires with triangular cross section

    Energy Technology Data Exchange (ETDEWEB)

    Duque, C.A., E-mail: cduque@fisica.udea.edu.co [Instituto de Física, Universidad de Antioquia, AA 1226, Medellín (Colombia); Mora-Ramos, M.E. [Instituto de Física, Universidad de Antioquia, AA 1226, Medellín (Colombia); Facultad de Ciencias, Universidad Autónoma del Estado de Morelos, Ave. Universidad 1001, CP 62209, Cuernavaca, Morelos, México (Mexico); Kasapoglu, E.; Ungan, F.; Yesilgul, U. [Cumhuriyet University, Physics Department, 58140 Sivas (Turkey); Sakiroglu, S. [Dokuz Eylül University, Physics Department, 35160 Buca, İzmir (Turkey); Sari, H. [Cumhuriyet University, Physics Department, 58140 Sivas (Turkey); Sökmen, I. [Dokuz Eylül University, Physics Department, 35160 Buca, İzmir (Turkey)

    2013-11-15

    The 1s-like and 2p-like donor impurity energy states are studied in a semiconductor quantum wire of equilateral triangular cross section as functions of the impurity position and the geometrical size of the structure. Linear and nonlinear coefficients for the optical absorption and relative refractive index change associated with 1s→2p transitions are calculated for both the x-polarization and y-polarization of the incident light. The results show a mixed effect of redshift and blueshift depending on the location of the donor atom. Also, strong nonlinear contributions to the optical absorption coefficient are obtained for both polarizations in the on-center impurity case. -- Highlights: • The 1s- and 2p-like impurity states in triangular quantum-well wires. • Optical absorption and relative refractive index changes are calculated. • Redshift and blueshift in the optical structures depend on the donor position. • Strong nonlinear contributions to the absorption coefficient have been obtained.

  14. Nonlinear optical properties of a three-electron quantum dot with account of the Rashba spin-orbit interaction

    Energy Technology Data Exchange (ETDEWEB)

    Hassanabadi, Hassan, E-mail: h.hasanabadi@shahroodut.ac.ir [Physics Department, Shahrood University of Technology, P.O. Box 3619995161-316, Shahrood (Iran, Islamic Republic of); Rahimov, Hamed [Physics Department, Shahrood University of Technology, P.O. Box 3619995161-316, Shahrood (Iran, Islamic Republic of); Lu Liangliang [Department of Physics, College of Physics and Electronic Engineering, Guangzhou University, Guangzhou 510006 (China); Wang Chao [Institute of Public Administration, Guangzhou University, Guangzhou 510006 (China)

    2012-05-15

    In this study, a detailed investigation of the nonlinear optical properties such as optical absorption and refractive index change associated with intersubband transitions in a three-electron quantum dot in two dimensions in the presence of the Rashba spin-orbit interaction has been carried out. We present the exact wave functions and energy levels of the system. Numerical results on typical GaAs/AlGaAs materials show that the decrease of the quantum dot radius blueshifts and amplifies the absorption coefficients as well as the refractive index changes, as expected. Additionally, an increase of the optical intensity and relaxation time considerably changes the absorption coefficients and the refractive index changes. - Highlights: Black-Right-Pointing-Pointer We consider a three-electron quantum dot in 2D in the presence of the Rashba spin-orbit interaction. Black-Right-Pointing-Pointer We present the exact wave functions and energy levels of the system. Black-Right-Pointing-Pointer We apply this model for GaAs/AlGaAs materials. Black-Right-Pointing-Pointer The detailed nonlinear optical properties have been investigated.

  15. Quantum noise and spatio-temporal pattern formation in nonlinear optics

    DEFF Research Database (Denmark)

    Bache, Morten

    2002-01-01

    -harmonic field, and the distinct peaks at the critical wave numbers reveal a quantum image. A microscopical model is suggested as a guide to understanding the processes involved in producing a classical pattern. Finally, the quantum nature of the correlations leads to spatial multimode nonclassical light, which......This work concerns analytical and numerical investigations of cavity enhanced x2 frequency conversion processes, specifically second-harmonic generation (SHG). We focus on how the transverse degrees of freedom affect the dynamics, where the interaction between nonlinearity and diffraction gives...... rise to spatially modulated structures, patterns. The two main parts of the thesis are the classical model and the quantum mechanical model, the latter being an extension of the former by including the inherent quantum fluctuations of light. From a theoretical point of view the classical dynamics...

  16. Nonlinear quantum optics in the (ultra)strong light-matter coupling

    OpenAIRE

    Sánchez-Burillo, Eduardo; García-Ripoll, Juan José; Martín-Moreno, Luis; Zueco, David

    2014-01-01

    The propagation of $N$ photons in one dimensional waveguides coupled to $M$ qubits is discussed, both in the strong and ultrastrong qubit-waveguide coupling. Special emphasis is placed on the characterisation of the nonlinear response and its linear limit for the scattered photons as a function of $N$, $M$, qubit inter distance and light-matter coupling. The quantum evolution is numerically solved via the Matrix Product States technique. Both the time evolution for the field and qubits is com...

  17. Quantum and semiclassical physics behind ultrafast optical nonlinearity in the midinfrared: the role of ionization dynamics within the field half cycle.

    Science.gov (United States)

    Serebryannikov, E E; Zheltikov, A M

    2014-07-25

    Ultrafast ionization dynamics within the field half cycle is shown to be the key physical factor that controls the properties of optical nonlinearity as a function of the carrier wavelength and intensity of a driving laser field. The Schrödinger-equation analysis of a generic hydrogen quantum system reveals universal tendencies in the wavelength dependence of optical nonlinearity, shedding light on unusual properties of optical nonlinearities in the midinfrared. For high-intensity low-frequency fields, free-state electrons are shown to dominate over bound electrons in the overall nonlinear response of a quantum system. In this regime, semiclassical models are shown to offer useful insights into the physics behind optical nonlinearity.

  18. Organic nonlinear optical materials

    Science.gov (United States)

    Umegaki, S.

    1987-01-01

    Recently, it became clear that organic compounds with delocalized pi electrons show a great nonlinear optical response. Especially, secondary nonlinear optical constants of more than 2 digits were often seen in the molecular level compared to the existing inorganic crystals such as LiNbO3. The crystallization was continuously tried. Organic nonlinear optical crystals have a new future as materials for use in the applied physics such as photomodulation, optical frequency transformation, opto-bistabilization, and phase conjugation optics. Organic nonlinear optical materials, e.g., urea, O2NC6H4NH2, I, II, are reviewed with 50 references.

  19. Quasi-phase-matched concurrent nonlinearities in periodically poled KTiOPO(4) for quantum computing over the optical frequency comb.

    Science.gov (United States)

    Pysher, Matthew; Bahabad, Alon; Peng, Peng; Arie, Ady; Pfister, Olivier

    2010-02-15

    We report the successful design and experimental implementation of three coincident nonlinear interactions, namely ZZZ (type 0), ZYY (type I), and YYZ/YZY (type II) second-harmonic generation of 780 nm light from a 1560 nm pump beam in a single, multigrating, periodically poled KTiOPO(4) crystal. The resulting nonlinear medium is the key component for making a scalable quantum computer over the optical frequency comb of a single optical parametric oscillator.

  20. Nonlinear optical properties of near-infrared region Ag2S quantum dots pumped by nanosecond laser pulses

    OpenAIRE

    Li-wei Liu; Si-yi Hu; Yin-ping Dou; Tian-hang Liu; Jing-quan Lin; Yue Wang

    2015-01-01

    This study investigates near-infrared region Ag2S quantum dots (QDs) and their nonlinear optical response under 532 nm nanosecond laser pulses. Our experimental result shows that nonlinear transmission is reduced from 0.084 to 0.04. The observed narrowing behavior of the output pulse width shows superior optical limiting. We discuss the physical mechanisms responsible for the nonlinear optical response of the QDs. The average size of the nanocrystals was 5.5 nm. Our results suggest the possib...

  1. Third-order non-linear optical susceptibilities in diffusion modified AlxGa1-xN/GaN single quantum well

    Science.gov (United States)

    Das, T.; Panda, M.; Panda, S.; Panda, B. K.

    2017-05-01

    In this work, the variation of optical properties in the AlGaN/GaN quantum well after thermal annealing is studied. The potential profile change of the quantum well resulting from the interdiffusion of Ga and Al atoms across the interface of the well and the barrier during the thermal treatments is assumed to follow Fick's law. The results show that the thermal annealing can induce an increase of the optical susceptibilities in the AlGaN/GaN quantum well. However the third-order nonlinear optical susceptibilities are red shifted with increasing in diffusion lengths.

  2. Fast response of the optical nonlinearity in a GaAs/AlGaAs asymmetric triple quantum well structure

    CERN Document Server

    Ahn, S H; Sawaki, N

    1999-01-01

    The time response of the optical nonlinear behavior in a GaAs/AlGaAs asymmetric triple quantum well structure is estimated by using a picosecond pump-probe method at 77 K. From the results of the transmission of the probe pulse as a function of the delay time at the excitation wavelengths, a rise time of 5 approx 10 ps and a fall time of 8 approx 16 ps are obtained. The nonlinear behavior is attributed to the triple resonance of the electronic states due to the build-up of the internal field induced by the separation of photo-excited electrons and holes. It is found that the rise time is determined by the tunneling transfer time of the electrons in the narrowest well to an adjacent well separated by a thin potential barrier.

  3. Non-linear optical response of an impurity in a cylindrical quantum dot under the action of a magnetic field

    Science.gov (United States)

    Portacio, Alfonso A.; Rodríguez, Boris A.; Villamil, Pablo

    2017-04-01

    The linear and nonlinear optical response in a cylindrical quantum dot (CQD) of GaAs / Ga0.6Al0.4 As with a donor impurity in a uniform magnetic field applied in the axial direction of the cylinder is studied theoretically. The calculations were carried out in approximations of effective mass and two-level quantum systems. Using the variational method, the binding energies and the wave functions of the 1s-like y 2pz-like states for different positions of the impurity inside the CQD were found. It was found that the binding energy is greatest in the center of the CQD and diminishes as the impurity moves radially and/or axially. The optical rectification, the change in the refractive index, and the optical absorption were studied as functions of the energy of a photon incident on the CQD and different intensities of the magnetic field, with an impurity located at various positions. It was found that in a CDQ with an impurity inside, the effect of the variation of the intensity of the magnetic field on the optical response is much less than the effect produced by the variation of the position of the impurity. The physical reason for this behavior is that in nanostructures with impurities the Coulomb confinement is stronger than the magnetic confinement. It was also found that when the impurity is in the center of the quantum dot, the optical rectification coefficient is zero, due to the symmetry that the wave function of the impurity exhibits at this geometric point. When the impurity moves in the axial direction, the symmetry is broken and the optical rectification coefficient is different from zero, and its value increases as the impurity moves away from the center of the CQD.

  4. Nonlinear optical rectification in a vertically coupled lens-shaped InAs/GaAs quantum dots with wetting layers under hydrostatic pressure and temperature

    Energy Technology Data Exchange (ETDEWEB)

    Ben Mahrsia, R.; Choubani, M., E-mail: mohsenchoubani3@yahoo.fr; Bouzaiene, L.; Maaref, H.

    2016-06-25

    In this paper we explore the structure parameters, hydrostatic pressure and temperature effects on Nonlinear optical rectification (NOR) in an asymmetric vertically coupled lens-shaped InAs/GaAs quantum dots. During epitaxial growth, lens-shaped quantum dots (QDs) are formed on the wetting layer (WL). Many theoretical works have neglected WL and its effect on nonlinear optical properties of QD-based systems for sake of simplicity. However, in this work the WL has been shown to be so influential in the intersubband energy and nonlinear optical rectification magnitude. Also, a detailed and comprehensive study of the nonlinear optical rectification is theoretical investigated within the framework of the compact density-matrix approach and finite difference method (FDM). It's found that nonlinear optical rectification coefficient is strongly affected not only by the WL, but also by the pressure, temperature and the coupled width between the QDs. Obtained results revealed that a red or a blue shift cane be observed. This behavior in the NOR gives a new degree of freedom in regions of interest for device applications. - Highlights: • Vertically coupled lens-shaped InAs/GaAs quantum dots is investigated. • Photon energy shifts towards the red with increasing pressure. • Photon energy shifts towards the blue with increasing temperature. • Intersubband energy decreases with increasing the wetting layer width. • Nonlinear optical rectification magnitude is controlled and adjusted.

  5. Nonlinear optical properties of free standing films of PbS quantum dots in the nonresonant femtosecond regime

    OpenAIRE

    Kurian, Pushpa Ann; Vijayan, C.; Nag, Amit; Goswami, Debabrata

    2007-01-01

    Devices based on optical technology for high speed communication networks require materials with large nonlinear optical response in the ultrafast regime. Nonlinear optical materials have also attracted wide attention as potential candidates for the protection of optical sensors and eyes while handling lasers. Optical limiters have a constant transmittance at low input influence and a decrease in transmittance at higher fluences and are based on a variety of mechanisms such as nonlinear refra...

  6. Nonlinear fiber optics

    CERN Document Server

    Agrawal, Govind P

    2001-01-01

    The Optical Society of America (OSA) and SPIE - The International Society for Optical Engineering have awarded Govind Agrawal with an honorable mention for the Joseph W. Goodman Book Writing Award for his work on Nonlinear Fiber Optics, 3rd edition.Nonlinear Fiber Optics, 3rd Edition, provides a comprehensive and up-to-date account of the nonlinear phenomena occurring inside optical fibers. It retains most of the material that appeared in the first edition, with the exception of Chapter 6, which is now devoted to the polarization effects relevant for light propagation in optical

  7. Stark effect-dependent of impurity-related nonlinear optical absorption of a (In,Ga)N-GaN spherical quantum dot

    Science.gov (United States)

    El Ghazi, Haddou; Zorkani, Izeddine; Jorio, Anouar

    2015-03-01

    The nonlinear intra-conduction band optical properties of a wurtzite (In,Ga)N-GaN spherical quantum dot are investigated. The linear, third-order nonlinear, and total absorption coefficients (ACs) of the 1s-1p transition are computed via a combination of the quantum genetic algorithm (QGA) and the Hartree-Fock-Roothaan (HFR) method. The external applied electric field effect is examined within the single-band effective mass and the one-parabolic-band approximations under a finite potential barrier. It is found that the electric field has a great impact on the optical properties of QDs: (i) a significant redshift of the resonant peak is obtained, (ii) the maximum of the amplitude of the optical total AC decreases nonlinearly, and (iii) the Stark shift increases nonlinearly, tending toward the saturation regime. Compared with findings, good agreement is shown.

  8. Non-linear optical processes involving excited subbands in laser-dressed quantum wires with triangular cross-section

    Science.gov (United States)

    Radu, A.; Duque, C. A.

    2015-08-01

    The conduction subband structure of a triangular cross-section GaAs/AlGaAs quantum well wire under intense laser field is theoretically investigated by taking into account a finite confining potential. The calculation of the subband energy levels is based on a two-dimensional finite element method within the effective mass approximation. It is shown that a transversally polarized laser field non-uniformly shifts the subband energy levels and could be used for tuning the intersubband transitions and altering the related optical susceptibilities. We found that the non-resonant laser field allows the magnification and the red- or blueshift of the third-order non-linear susceptibility peaks for particular polarizations of the pump light and proper laser parameter values. The effects of the laser dressing field on the intersubband third harmonic generation and quadratic electro-optical process are discussed.

  9. Multiphoton quantum optics and quantum state engineering

    Energy Technology Data Exchange (ETDEWEB)

    Dell' Anno, Fabio [Dipartimento di Fisica ' E. R. Caianiello' , Universita degli Studi di Salerno, CNISM and CNR-INFM Coherentia, and INFN Sezione di Napoli, Gruppo Collegato di Salerno, Via S. Allende, I-84081 Baronissi (Saudi Arabia) (Italy)]. E-mail: dellanno@sa.infn.it; De Siena, Silvio [Dipartimento di Fisica ' E. R. Caianiello' , Universita degli Studi di Salerno, CNISM and CNR-INFM Coherentia, and INFN Sezione di Napoli, Gruppo Collegato di Salerno, Via S. Allende, I-84081 Baronissi (SA) (Italy)]. E-mail: desiena@sa.infn.it; Illuminati, Fabrizio [Dipartimento di Fisica ' E. R. Caianiello' , Universita degli Studi di Salerno, CNISM and CNR-INFM Coherentia, and INFN Sezione di Napoli, Gruppo Collegato di Salerno, Via S. Allende, I-84081 Baronissi (SA) (Italy)]. E-mail: illuminati@sa.infn.it

    2006-05-15

    We present a review of theoretical and experimental aspects of multiphoton quantum optics. Multiphoton processes occur and are important for many aspects of matter-radiation interactions that include the efficient ionization of atoms and molecules, and, more generally, atomic transition mechanisms; system-environment couplings and dissipative quantum dynamics; laser physics, optical parametric processes, and interferometry. A single review cannot account for all aspects of such an enormously vast subject. Here we choose to concentrate our attention on parametric processes in nonlinear media, with special emphasis on the engineering of nonclassical states of photons and atoms that are relevant for the conceptual investigations as well as for the practical applications of forefront aspects of modern quantum mechanics. We present a detailed analysis of the methods and techniques for the production of genuinely quantum multiphoton processes in nonlinear media, and the corresponding models of multiphoton effective interactions. We review existing proposals for the classification, engineering, and manipulation of nonclassical states, including Fock states, macroscopic superposition states, and multiphoton generalized coherent states. We introduce and discuss the structure of canonical multiphoton quantum optics and the associated one- and two-mode canonical multiphoton squeezed states. This framework provides a consistent multiphoton generalization of two-photon quantum optics and a consistent Hamiltonian description of multiphoton processes associated to higher-order nonlinearities. Finally, we discuss very recent advances that by combining linear and nonlinear optical devices allow to realize multiphoton entangled states of the electromagnetic field, either in discrete or in continuous variables, that are relevant for applications to efficient quantum computation, quantum teleportation, and related problems in quantum communication and information.

  10. Metal colloids and semiconductor quantum dots: Linear and nonlinear optical properties

    Science.gov (United States)

    Henderson, D. O.; My, R.; Tung, Y.; Ueda, A.; Zhu, J.; Collins, W. E.; Hall, Christopher

    1995-01-01

    One aspect of this project involves a collaborative effort with the Solid State Division of ORNL. The thrust behind this research is to develop ion implantion for synthesizing novel materials (quantum dots wires and wells, and metal colloids) for applications in all optical switching devices, up conversion, and the synthesis of novel refractory materials. In general the host material is typically a glass such as optical grade silica. The ions of interest are Au, Ag, Cd, Se, In, P, Sb, Ga and As. An emphasis is placed on host guest interactions between the matrix and the implanted ion and how the matrix effects and implantation parameters can be used to obtain designer level optical devices tailored for specific applications. The specific materials of interest are: CdSe, CdTe, InAs, GaAs, InP, GaP, InSb, GaSb and InGaAs. A second aspect of this research program involves using porous glass (25-200 A) for fabricating materials of finite size. In this part of the program, we are particularly interested in characterizing the thermodynamic and optical properties of these non-composite materials. We also address how phase diagram of the confined material is altered by the interfacial properties between the confined material and the pore wall.

  11. Metal colloids and semiconductor quantum dots: Linear and nonlinear optical properties

    Science.gov (United States)

    Henderson, D. O.; My, R.; Tung, Y.; Ueda, A.; Zhu, J.; Collins, W. E.; Hall, Christopher

    1995-01-01

    One aspect of this project involves a collaborative effort with the Solid State Division of ORNL. The thrust behind this research is to develop ion implantion for synthesizing novel materials (quantum dots wires and wells, and metal colloids) for applications in all optical switching devices, up conversion, and the synthesis of novel refractory materials. In general the host material is typically a glass such as optical grade silica. The ions of interest are Au, Ag, Cd, Se, In, P, Sb, Ga and As. An emphasis is placed on host guest interactions between the matrix and the implanted ion and how the matrix effects and implantation parameters can be used to obtain designer level optical devices tailored for specific applications. The specific materials of interest are: CdSe, CdTe, InAs, GaAs, InP, GaP, InSb, GaSb and InGaAs. A second aspect of this research program involves using porous glass (25-200 A) for fabricating materials of finite size. In this part of the program, we are particularly interested in characterizing the thermodynamic and optical properties of these non-composite materials. We also address how phase diagram of the confined material is altered by the interfacial properties between the confined material and the pore wall.

  12. Distributed nonlinear optical response

    DEFF Research Database (Denmark)

    Nikolov, Nikola Ivanov

    2005-01-01

    The purpose of the research presented here is to investigate basic physical properties in nonlinear optical materials with delayed or nonlocal nonlinearity. Soliton propagation, spectral broadening and the influence of the nonlocality or delay of the nonlinearity are the main focusses in the work...

  13. Nonlinear optical materials.

    Science.gov (United States)

    Eaton, D F

    1991-07-19

    The current state of materials development in nonlinear optics is summarized, and the promise of these materials is critically evaluated. Properties and important materials constants of current commercial materials and of new, promising, inorganic and organic molecular and polymeric materials with potential in second- and third-order nonlinear optical applications are presented.

  14. Steady-state linear optical properties and Kerr nonlinear optical response of a four-level quantum dot with phonon-assisted transition

    Science.gov (United States)

    Yan-Chao, She; Ting-Ting, Luo; Wei-Xi, Zhang; Mao-Wu, Ran; Deng-Long, Wang

    2016-01-01

    The linear optical properties and Kerr nonlinear optical response in a four-level loop configuration GaAs/AlGaAs semiconductor quantum dot are analytically studied with the phonon-assisted transition (PAT). It is shown that the changes among a single electromagnetically induced transparency (EIT) window, a double EIT window and the amplification of the probe field in the absorption curves can be controlled by varying the strength of PAT κ. Meanwhile, double switching from the anomalous dispersion regime to the normal dispersion regime can likely be achieved by increasing the Rabi energy of the external optical control field. Furthermore, we demonstrate that the group velocity of the probe field can be practically regulated by varying the PAT and the intensity of the optical control field. In the nonlinear case, it is shown that the large SPM and XPM can be achieved as linear absorption vanishes simultaneously, and the PAT can suppress both third-order self-Kerr and the cross-Kerr nonlinear effect of the QD. Our study is much more practical than its atomic counterpart due to its flexible design and the controllable interference strength, and may provide some new possibilities for technological applications. Project supported by the National Natural Science Foundation of China (Grant No. 61367003), the Scientific Research Fund of Hunan Provincial Education Department, China (Grant No. 12A140), and the Scientific Research Fund of Guizhou Provincial Education Department, China (Grant Nos. KY[2015]384 and KY[2015]446).

  15. Nonlinear optics and photonics

    CERN Document Server

    He, Guang S

    2015-01-01

    This book provides a comprehensive presentation on most of the major topics in nonlinear optics and photonics, with equal emphasis on principles, experiments, techniques, and applications. It covers many major new topics including optical solitons, multi-photon effects, nonlinear photoelectric effects, fast and slow light , and Terahertz photonics. Chapters 1-10 present the fundamentals of modern nonlinear optics, and could be used as a textbook with problems provided at the end of each chapter. Chapters 11-17 cover the more advanced topics of techniques and applications of nonlinear optics and photonics, serving as a highly informative reference for researchers and experts working in related areas. There are also 16 pages of color photographs to illustrate the visual appearances of some typical nonlinear optical effects and phenomena. The book could be adopted as a textbook for both undergraduates and graduate students, and serve as a useful reference work for researchers and experts in the fields of physics...

  16. A high repetition rate experimental setup for quantum non-linear optics with cold Rydberg atoms

    Science.gov (United States)

    Busche, Hannes; Ball, Simon W.; Huillery, Paul

    2016-12-01

    Using electromagnetically induced transparency and photon storage, the strong dipolar interactions between Rydberg atoms and the resulting dipole blockade can be mapped onto light fields to realise optical non-linearities and interactions at the single photon level. We report on the realisation of an experimental apparatus designed to study interactions between single photons stored as Rydberg excitations in optically trapped microscopic ensembles of ultracold 87Rb atoms. A pair of in-vacuum high numerical aperture lenses focus excitation and trapping beams down to 1 μm, well below the Rydberg blockade. Thanks to efficient magneto-optical trap (MOT) loading from an atomic beam generated by a 2D MOT and the ability to recycle the microscopic ensembles more than 20000 times without significant atom loss, we achieve effective repetition rates exceeding 110 kHz to obtain good photon counting statistics on reasonable time scales. To demonstrate the functionality of the setup, we present evidence of strong photon interactions including saturation of photon storage and the retrieval of non-classical light. Using in-vacuum antennae operating at up to 40 GHz, we perform microwave spectroscopy on photons stored as Rydberg excitations and observe an interaction induced change in lineshape depending on the number of stored photons.

  17. Nonlinear Optical Properties of Novel Mono-O-Hydroxy Bidentate Schiff Base: Quantum Chemical Calculations

    Directory of Open Access Journals (Sweden)

    N. S. Labidi

    2013-01-01

    Full Text Available The semiempirical AM1 SCF method is used to study the first static hyperpolarizabilities β of some novel mono-O-Hydroxy bidentate Schiff base in which electron donating (D and electron accepting (A groups were introduced on either side of the Schiff base ring system. Geometries of all molecules were optimized at the semiempirical AM1. The first static hyperpolarizabilities of these molecules were calculated using Hyperchem package. To understand this phenomenon in the context of molecular orbital picture, we examined the molecular HOMO and molecular LUMO generated via Hyperchem. The study reveals that the mono-O-Hydroxy bidentate Schiff bases have large β values and hence in general may have potential applications in the development of nonlinear optical materials.

  18. Quantum optics for experimentalists

    CERN Document Server

    Ou, Zhe-Yu Jeff

    2017-01-01

    This book on quantum optics is from the point of view of an experimentalist. It approaches the theory of quantum optics with the language of optical modes of classical wave theory, with which experimentalists are most familiar.

  19. Linear and nonlinear optical absorption coefficients and refractive index changes associated with intersubband transitions in a quantum disk with flat cylindrical geometry

    Energy Technology Data Exchange (ETDEWEB)

    Gambhir, Monica, E-mail: monica.gambhir@yahoo.com [Department of Physics and Astrophysics, University of Delhi, Delhi 110007 (India); Kumar, Manoj [Department of Physics and Astrophysics, University of Delhi, Delhi 110007 (India); Jha, P.K. [Department of Physics and Astrophysics, University of Delhi, Delhi 110007 (India); Deen Dayal Upadhyaya College, University of Delhi, Delhi 110015 (India); Mohan, Man [Department of Physics and Astrophysics, University of Delhi, Delhi 110007 (India)

    2013-11-15

    The linear and nonlinear optical absorption coefficients and changes in the refractive index in GaAs/AlGaAs quantum disk in the form of a flat cylinder are investigated theoretically in the presence of a static magnetic and a laser field within the framework of the compact-density matrix approach. It is found that the absorption coefficients and the refractive index changes depend not only on the optical wave intensity but also on the strength of the static magnetic field. The intersubband relaxation time, also, has an important influence on the linear and nonlinear optical properties of a quantum disk. -- Highlights: • The study is carried out in a quantum disk having quantum dot geometry. • The linear and non-linear optical properties are studied using density matrix approach. • The study is carried out in the presence of a laser field and a magnetic field. • Influence of incident photon energy and static magnetic field is analyzed. • The optical properties are found to be greatly influenced by the relaxation time.

  20. Linear and nonlinear optical properties of functionalized CdSe quantum dots prepared by plasma sputtering and wet chemistry.

    Science.gov (United States)

    Humbert, Christophe; Dahi, Abdellatif; Dalstein, Laetitia; Busson, Bertrand; Lismont, Marjorie; Colson, Pierre; Dreesen, Laurent

    2015-05-01

    We develop an innovative manufacturing process, based on radio-frequency magnetron sputtering (RFMS), to prepare neat CdSe quantum dots (QDs) on glass and silicon substrates and further chemically functionalize them. In order to validate the fabrication protocol, their optical properties are compared with those of QDs obtained from commercial solutions and deposited by wet chemistry on the substrates. Firstly, AFM measurements attest that nano-objects with a mean diameter around 13 nm are located on the substrate after RFMS treatment. Secondly, the UV-Vis absorption study of this deposited layer shows a specific optical absorption band, located at 550 nm, which is related to a discrete energy level of QDs. Thirdly, by using two-color sum-frequency generation (2C-SFG) nonlinear optical spectroscopy, we show experimentally the functionalization efficiency of the RFMS CdSe QDs layer with thiol derived molecules, which is not possible on the QDs layer prepared by wet chemistry due to the surfactant molecules from the native solution. Finally, 2C-SFG spectroscopy, performed at different visible wavelengths, highlights modifications of the vibration mode shape whatever the QDs deposition method, which is correlated to the discrete energy level of the QDs.

  1. Nonlinear Optical Rectennas

    CERN Document Server

    Stolz, A; Markey, L; Francs, G Colas des; Bouhelier, A

    2013-01-01

    We introduce strongly-coupled optical gap antennas to interface optical radiation with current-carrying electrons at the nanoscale. The transducer relies on the nonlinear optical and electrical properties of an optical antenna operating in the tunneling regime. We discuss the underlying physical mechanisms controlling the conversion and demonstrate that a two-wire optical antenna can provide advanced optoelectronic functionalities beyond tailoring the electromagnetic response of a single emitter. Interfacing an electronic command layer with a nanoscale optical device may thus be facilitated by the optical rectennas discussed here.

  2. Composition dependent structural, Raman and nonlinear optical properties of PVA capped Zn1-x-yCdxCuyS quantum dots

    Science.gov (United States)

    Vineeshkumar, T. V.; Rithesh Raj, D.; Prasanth, S.; Sankar, Pranitha; Unnikrishnan, N. V.; Mahadevan Pillai, V. P.; Sudarsanakumar, C.

    2016-08-01

    Composition dependent structural, optical nonlinear and limiting properties of PVA capped Zn1-x-yCdxCuyS quantum dots at different Cu:Zn ratio synthesized by insitu technique is subjected to detailed investigation. Cubic phase of the quantum dots were identified from XRD with particle size in the range 2.5 nm-3.5 nm find excellent correlation with the particle size measured from TEM. With increase in Cu concentration: systematic increment in lattice parameter, red shift in absorption edges and luminescence quenching is observed. Raman scattering reveals good photoactivity evidenced by intensity variation and shifting of LO and TO phonon modes. The intensity dependent third order nonlinearity is studied using Q switched Nd: YAG laser with 532 nm irradiation. Progressive increase in 3 PA coefficient indicated that prepared samples exhibit good nonlinear and optical limiting properties.

  3. Linear and nonlinear optical absorption coefficients and refractive index changes in modulation-doped quantum wells: Effects of the magnetic field and hydrostatic pressure

    Energy Technology Data Exchange (ETDEWEB)

    Nazari, M.; Karimi, M.J., E-mail: karimi@sutech.ac.ir; Keshavarz, A.

    2013-11-01

    In this study, the linear, the third-order nonlinear and total optical absorption coefficients and refractive index changes of a modulation-doped GaAs/Al{sub x}Ga{sub 1−x}As quantum well are investigated numerically. In the effective-mass approximation, the electronic structure of modulation-doped quantum well is calculated by solving the Schrödinger and Poisson equations self-consistently. Optical properties are obtained using the compact density matrix approach. The effects of structure parameters, the applied magnetic field and the hydrostatic pressure on the optical properties of the modulation-doped quantum well are studied. Results show that the resonant peaks shift toward the higher (lower) energies with the increase in the magnetic field (pressure). The magnitude of the resonant peaks of the optical properties decreases with the increasing magnetic field or pressure.

  4. Optical bistability at 980 nm in a strained InGaAs/GaAs multiple quantum well microcavity with resonant periodic nonlinearity

    Science.gov (United States)

    Pellat, D.; Azoulay, R.; Leroux, G.; Dugrand, L.; Raffle, Y.; Kuszelewicz, R.; Oudar, J. L.

    1993-05-01

    We report on a novel monolithic all-optical bistable device operating at 980 nm, based on the dispersive optical nonlinearity of strained InGaAs/GaAs quantum wells located at the antinodes of the microcavity optical field. This design maximizes the interaction with the intracavity field, and allowed the use of only twelve quantum wells of 10 nm thickness. The first observation of all-optical bistability with strained InGaAs/GaAs quantum wells is reported, with a contrast ratio of 7:1 and a threshold intensity of 1 kW/sq cm. The operating wavelength offers such key advantages as substrate transparency and compatibility with vertical cavity surface emitting lasers.

  5. Multiphoton Quantum Optics and Quantum State Engineering

    CERN Document Server

    Dell'Anno, F; Illuminati, F; 10.1016/j.physrep.2006.01.004

    2009-01-01

    We present a review of theoretical and experimental aspects of multiphoton quantum optics. Multiphoton processes occur and are important for many aspects of matter-radiation interactions that include the efficient ionization of atoms and molecules, and, more generally, atomic transition mechanisms; system-environment couplings and dissipative quantum dynamics; laser physics, optical parametric processes, and interferometry. A single review cannot account for all aspects of such an enormously vast subject. Here we choose to concentrate our attention on parametric processes in nonlinear media, with special emphasis on the engineering of nonclassical states of photons and atoms. We present a detailed analysis of the methods and techniques for the production of genuinely quantum multiphoton processes in nonlinear media, and the corresponding models of multiphoton effective interactions. We review existing proposals for the classification, engineering, and manipulation of nonclassical states, including Fock states...

  6. Effects of applied electric and magnetic fields on the nonlinear optical rectification and second-harmonic generation in a graded quantum well under intense laser field

    Science.gov (United States)

    Ungan, Fatih

    2017-01-01

    In this present study, the effects of electric and magnetic fields on the nonlinear optical rectification and second-harmonic generation in a graded quantum well under intense laser field have been investigated theoretically. The energy eigenvalues and their corresponding eigenfunctions are obtained by solving Schrödinger equation within the framework of effective mass approximation. The analytic expressions for the optical properties are calculated by the compact-density-matrix approach and iterative method. The numerical results are presented for a typical GaAs/Ga1- x Al x As quantum well. The results show that the nonlinear optical rectification and second-harmonic generation coefficients are considerably affected by the electromagnetic fields and intense laser field.

  7. Ultrafast nonlinear optics

    CERN Document Server

    Leburn, Christopher; Reid, Derryck

    2013-01-01

    The field of ultrafast nonlinear optics is broad and multidisciplinary, and encompasses areas concerned with both the generation and measurement of ultrashort pulses of light, as well as those concerned with the applications of such pulses. Ultrashort pulses are extreme events – both in terms of their durations, and also the high peak powers which their short durations can facilitate. These extreme properties make them powerful experiment tools. On one hand, their ultrashort durations facilitate the probing and manipulation of matter on incredibly short timescales. On the other, their ultrashort durations can facilitate high peak powers which can drive highly nonlinear light-matter interaction processes. Ultrafast Nonlinear Optics covers a complete range of topics, both applied and fundamental in nature, within the area of ultrafast nonlinear optics. Chapters 1 to 4 are concerned with the generation and measurement of ultrashort pulses. Chapters 5 to 7 are concerned with fundamental applications of ultrasho...

  8. Exploring electro-optic effect and third-order nonlinear optical susceptibility of impurity doped quantum dots: Interplay between hydrostatic pressure, temperature and noise

    Science.gov (United States)

    Ganguly, Jayanta; Saha, Surajit; Bera, Aindrila; Ghosh, Manas

    2017-03-01

    We study the profiles of electro-optic effect (EOE) and third-order nonlinear optical susceptibility (TONOS) of impurity doped GaAs quantum dots (QDs) under the combined influence of hydrostatic pressure (HP) and temperature (T) taking into account the presence of Gaussian white noise. Noise has been introduced to the system additively and multiplicatively. The doped dot has been subjected to a polarized monochromatic electromagnetic field. Effect of application of noise is elegantly reflected through prominent change of peak shift (blue/red) and variation of peak height (increase/ıdecrease) of above nonlinear optical (NLO) properties as temperature and pressure are varied over a range. Interestingly, all such changes subtly depend on mode of application (additive/multiplicative) of noise. The noteworthy influence of the interplay between noise strength and its mode of application on the said NLO properties has also been critically scrutinized. The findings highlight remarkable role played by noise in tuning above NLO properties of doped QD system under the prominent presence of both hydrostatic pressure and temperature.

  9. Nonlinear effects in optical fibers

    CERN Document Server

    Ferreira, Mario F

    2011-01-01

    Cutting-edge coverage of nonlinear phenomena occurring inside optical fibers Nonlinear fiber optics is a specialized part of fiber optics dealing with optical nonlinearities and their applications. As fiber-optic communication systems have become more advanced and complex, the nonlinear effects in optical fibers have increased in importance, as they adversely affect system performance. Paradoxically, the same nonlinear phenomena also offer the promise of addressing the bandwidth bottleneck for signal processing for future ultra-high speed optical networks. Nonlinear Effects in Optical Fiber

  10. Optical Quantum Computing

    National Research Council Canada - National Science Library

    Jeremy L. O'Brien

    2007-01-01

    In 2001, all-optical quantum computing became feasible with the discovery that scalable quantum computing is possible using only single-photon sources, linear optical elements, and single-photon detectors...

  11. Effects of magnetic field on the terahertz nonlinear optical properties in donor-doped GaAs/AlGaAs quantum wells

    Energy Technology Data Exchange (ETDEWEB)

    Yildirim, Hasan [Faculty of Science, Department of Physics, Karabuek University, Karabuek 78050 (Turkey); Aslan, Bulent [Faculty of Science, Department of Physics, Anadolu University, Yunus Emre Campus, Eskisehir 26470 (Turkey)

    2012-11-15

    Effects of the magnetic field on nonlinear optical properties at THz range in GaAs/AlGaAs quantum wells doped with donor atoms are investigated. Expressions for the third-order nonlinear optical susceptibilities are obtained through the solution of the density matrix equations of motion within the rotating wave approximation. Donor binding energies are calculated variationally by means of an iterative shooting algorithm. Magnetic field has strong effect on the nonlinear susceptibility: it removes the degeneracy in energies of 2p{sub {+-}} impurity states and increases the absolute value of the nonlinearity. It is also shown that a large and tunable optical nonlinear figure of merit is possible with the magnetic field applied in the growth direction. The nonlinear optical quantities are also calculated for donor distributions with different full width at half maximum values in the absence of magnetic field and the observed features at low energy part are attributed to the increasing homogeneity in the donor distribution. (Copyright copyright 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  12. Mesoscale Engineering of Nanocomposite Nonlinear Optical Materials

    Energy Technology Data Exchange (ETDEWEB)

    Afonso, C.N.; Feldman, L.C.; Gonella, F.; Haglund, R.F.; Luepke, G.; Magruder, R.H.; Mazzoldi, P.; Osborne, D.H.; Solis, J.; Zuhr, R.A.

    1999-11-01

    Complex nonlinear optical materials comprising elemental, compound or alloy quantum dots embedded in appropriate dielectric or semiconducting hosts may be suitable for deployment in photonic devices. Ion implantation, ion exchange followed by ion implantation, and pulsed laser deposition have ail been used to synthesize these materials. However, the correlation between the parameters of energetic-beam synthesis and the nonlinear optical properties is still very rudimentary when one starts to ask what is happening at nanoscale dimensions. Systems integration of complex nonlinear optical materials requires that the mesoscale materials science be well understood within the context of device structures. We discuss the effects of beam energy and energy density on quantum-dot size and spatial distribution, thermal conductivity, quantum-dot composition, crystallinity and defects - and, in turn, on the third-order optical susceptibility of the composite material. Examples from recent work in our laboratories are used to illustrate these effects.

  13. Linearizing nonlinear optics

    CERN Document Server

    Schmidt, Bruno E; Ernotte, Guilmot; Clerici, Matteo; Morandotti, Roberto; Ibrahim, Heide; Legare, Francois

    2016-01-01

    In the framework of linear optics, light fields do not interact with each other in a medium. Yet, when their field amplitude becomes comparable to the electron binding energies of matter, the nonlinear motion of these electrons emits new dipole radiation whose amplitude, frequency and phase differ from the incoming fields. Such high fields are typically achieved with ultra-short, femtosecond (1fs = 10-15 sec.) laser pulses containing very broad frequency spectra. Here, the matter not only couples incoming and outgoing fields but also causes different spectral components to interact and mix through a convolution process. In this contribution, we describe how frequency domain nonlinear optics overcomes the shortcomings arising from this convolution in conventional time domain nonlinear optics1. We generate light fields with previously inaccessible properties because the uncontrolled coupling of amplitudes and phases is turned off. For example, arbitrary phase functions are transferred linearly to the second har...

  14. Fundamentals of nonlinear optics

    CERN Document Server

    Powers, Peter E

    2011-01-01

    Peter Powers's rigorous but simple description of a difficult field keeps the reader's attention throughout. … All chapters contain a list of references and large numbers of practice examples to be worked through. … By carefully working through the proposed problems, students will develop a sound understanding of the fundamental principles and applications. … the book serves perfectly for an introductory-level course for second- and third-order nonlinear optical phenomena. The author's writing style is refreshing and original. I expect that Fundamentals of Nonlinear Optics will fast become pop

  15. Structure versus solvent effects on nonlinear optical properties of push-pull systems: a quantum-mechanical study based on a polarizable continuum model.

    Science.gov (United States)

    Corozzi, Alessandro; Mennucci, Benedetta; Cammi, Roberto; Tomasi, Jacopo

    2009-12-31

    A quantum mechanical investigation on the effects of the solvent and the structure on nonlinear optical activity of a class of merocyanine compounds has been conducted. The interplay of the two effects on the first hyperpolarizability, computed at density functional theory and second-order Møller-Plesset level, has been analyzed in combination with ground state properties and geometries and excited state energies and dipoles. A critical analysis of the simplified two-level model has also been presented.

  16. Effect of size and indium-composition on linear and nonlinear optical absorption of InGaN/GaN lens-shaped quantum dot

    Science.gov (United States)

    Ahmed, S. Jbara; Zulkafli, Othaman; M, A. Saeed

    2016-05-01

    Based on the Schrödinger equation for envelope function in the effective mass approximation, linear and nonlinear optical absorption coefficients in a multi-subband lens quantum dot are investigated. The effects of quantum dot size on the interband and intraband transitions energy are also analyzed. The finite element method is used to calculate the eigenvalues and eigenfunctions. Strain and In-mole-fraction effects are also studied, and the results reveal that with the decrease of the In-mole fraction, the amplitudes of linear and nonlinear absorption coefficients increase. The present computed results show that the absorption coefficients of transitions between the first excited states are stronger than those of the ground states. In addition, it has been found that the quantum dot size affects the amplitudes and peak positions of linear and nonlinear absorption coefficients while the incident optical intensity strongly affects the nonlinear absorption coefficients. Project supported by the Ministry of Higher Education and Scientific Research in Iraq, Ibnu Sina Institute and Physics Department of Universiti Teknologi Malaysia (UTM RUG Vote No. 06-H14).

  17. Fabricating third-order nonlinear optical susceptibility of impurity doped quantum dots in the presence of Gaussian white noise

    Science.gov (United States)

    Ganguly, Jayanta; Saha, Surajit; Pal, Suvajit; Ghosh, Manas

    2016-03-01

    We perform a meticulous analysis of profiles of third-order nonlinear optical susceptibility (TONOS) of impurity doped quantum dots (QDs) in the presence and absence of noise. We have invoked Gaussian white noise in the present study and noise has been introduced to the system additively and multiplicatively. The QD is doped with a Gaussian impurity. A magnetic field applied perpendicularly serves as a confinement source and the doped system has been exposed to a static external electric field. The TONOS profiles have been monitored against a continuous variation of incident photon energy when several important parameters such as electric field strength, magnetic field strength, confinement energy, dopant location, Al concentration, dopant potential, relaxation time, anisotropy, and noise strength assume different values. Moreover, the influence of mode of introduction of noise (additive/multiplicative) on the TONOS profiles has also been addressed. The said profiles are found to be consisting of interesting observations such as shift of TONOS peak position and maximization/minimization of TONOS peak intensity. The presence of noise alters the features of TONOS profiles and sometimes enhances the TONOS peak intensity from that of noise-free state. Furthermore, the mode of application of noise also often tailors the TONOS profiles in diverse fashions. The observations accentuate the possibility of tuning the TONOS of doped QD systems in the presence of noise.

  18. PREFACE: Quantum Optics III

    Science.gov (United States)

    Orszag, M.; Retamal, J. C.; Saavedra, C.; Wallentowitz, S.

    2007-06-01

    All the 50 years of conscious pondering did not bring me nearer to an answer to the question `what is light quanta?'. Nowadays, every rascal believes, he knows it, however, he is mistaken. (A Einstein, 1951 in a letter to M Besso) Quantum optics has played a key role in physics in the last several decades. On the other hand, in these early decades of the information age, the flow of information is becoming more and more central to our daily life. Thus, the related fields of quantum information theory as well as Bose-Einstein condensation have acquired tremendous importance in the last couple of decades. In Quantum Optics III, a fusion of these fields appears in a natural way. Quantum Optics III was held in Pucón, Chile, in 27-30 of November, 2006. This beautiful location in the south of Chile is near the lake Villarrica and below the snow covered volcano of the same name. This fantastic environment contributed to a relaxed atmosphere, suitable for informal discussion and for the students to have a chance to meet the key figures in the field. The previous Quantum Optics conferences took place in Santiago, Chile (Quantum Optics I, 2000) and Cozumel, Mexico (Quantum Optics II, 2004). About 115 participants from 19 countries attended and participated in the meeting to discuss a wide variety of topics such as quantum-information processing, experiments related to non-linear optics and squeezing, various aspects of entanglement including its sudden death, correlated twin-photon experiments, light storage, decoherence-free subspaces, Bose-Einstein condensation, discrete Wigner functions and many more. There was a strong Latin-American participation from Argentina, Brazil, Chile, Colombia, Peru, Uruguay, Venezuela and Mexico, as well as from Europe, USA, China, and Australia. New experimental and theoretical results were presented at the conference. In Latin-America a quiet revolution has taken place in the last twenty years. Several groups working in quantum optics and

  19. Intense laser field effects on the linear and nonlinear intersubband optical properties in a strained InGaN/GaN quantum well

    Energy Technology Data Exchange (ETDEWEB)

    Karimi, M.J., E-mail: karimi@sutech.ac.ir; Vafaei, H.

    2014-11-01

    In this work, the linear, the third-order nonlinear and the total optical absorption coefficients and refractive index changes of a strained InGaN/GaN quantum well are investigated numerically. In the effective-mass approximation, the electronic energy levels and the corresponding wave functions are calculated by taking into account the effects of spontaneous and piezoelectric polarization fields on the conduction band edge. Effects of intense laser field, In composition and the well width on the optical properties of the strained quantum well are studied. Results indicate that the laser field as well as the strain induced piezoelectric field considerably affects the confining potential of the quantum well. Results also show that the resonant peaks experience a red-shift (blue-shift) with the increase in the laser field intensity and well width (In composition)

  20. Nonlinear fibre optics overview

    DEFF Research Database (Denmark)

    Travers, J. C.; Frosz, Michael Henoch; Dudley, J. M.

    2010-01-01

    , provides a background to the associated nonlinear optical processes, treats the generation mechanisms from continuous wave to femtosecond pulse pump regimes and highlights the diverse applications. A full discussion of numerical methods and comprehensive computer code are also provided, enabling readers...

  1. Elements of quantum optics

    CERN Document Server

    Meystre, Pierre

    2007-01-01

    Elements of Quantum Optics gives a self-contained and broad coverage of the basic elements necessary to understand and carry out research in laser physics and quantum optics, including a review of basic quantum mechanics and pedagogical introductions to system-reservoir interactions and to second quantization. The text reveals the close connection between many seemingly unrelated topics, such as probe absorption, four-wave mixing, optical instabilities, resonance fluorescence and squeezing. It also comprises discussions of cavity quantum electrodynamics and atom optics. The 4th edition includes a new chapter on quantum entanglement and quantum information, as well as added discussions of the quantum beam splitter, electromagnetically induced transparency, slow light, and the input-output formalism needed to understand many problems in quantum optics. It also provides an expanded treatment of the minimum-coupling Hamiltonian and a simple derivation of the Gross-Pitaevskii equation, an important gateway to rese...

  2. Nonlinear optical rectification and the second and third harmonic generation in Pöschl–Teller quantum well under the intense laser field

    Energy Technology Data Exchange (ETDEWEB)

    Şakiroğlu, S., E-mail: serpil.sakiroglu@deu.edu.tr [Physics Department, Faculty of Science, Dokuz Eylül University, 35160 İzmir (Turkey); Ungan, F.; Yesilgul, U. [Physics Department, Faculty of Science, Cumhuriyet University, 58140 Sivas (Turkey); Mora-Ramos, M.E. [Facultad de Ciencias, Universidad Autónoma del Estado de Morelos, Ave. Universidad 1001, CP. 62209 Cuernavaca, Morelos (Mexico); Duque, C.A. [Instituto de Física, Universidad de Antioquia, AA 1226 Medellín (Colombia); Kasapoglu, E.; Sari, H. [Physics Department, Faculty of Science, Cumhuriyet University, 58140 Sivas (Turkey); Sökmen, İ. [Physics Department, Faculty of Science, Dokuz Eylül University, 35160 İzmir (Turkey)

    2012-05-07

    In this work, the effect of a non-resonant intense laser field on the optical rectification and second and third harmonic generation in a Pöschl–Teller quantum well is theoretically investigated. In this regard, the coefficients of nonlinear optical rectification and second and third harmonic generation are obtained by using the compact-density matrix approach and an iterative method. Different values of the asymmetry parameters of the Pöschl–Teller potential as well as intense laser field strength have been considered. Numerical results presented for a typical GaAs quantum wells show that higher-order optical effects are considerably sensitive to intense laser field and can be adjusted by a correct choice of asymmetry parameters of the potential. -- Highlights: ► Higher-order optical effects are considerably sensitive to the intense laser field. ► Increasing ILF shifts the maximum peaks of NOR, SHG and THG toward higher-energies. ► NOR and SHG increase with an enhancement in the asymmetry of the quantum well. ► Nonlinearities can be adjusted by a correct choice of asymmetry parameters.

  3. Role of surface states and defects in the ultrafast nonlinear optical properties of CuS quantum dots

    Energy Technology Data Exchange (ETDEWEB)

    Mary, K. A. Ann; Unnikrishnan, N. V., E-mail: nvu100@yahoo.com [School of Pure and Applied Physics, Mahatma Gandhi University, Kottayam 686560 (India); Philip, Reji [Light and Matter Physics Group, Raman Research Institute, C.V. Raman Avenue, Sadashivanagar, Bangalore 560080 (India)

    2014-07-01

    We report facile preparation of water dispersible CuS quantum dots (2–4 nm) and nanoparticles (5–11 nm) through a nontoxic, green, one-pot synthesis method. Optical and microstructural studies indicate the presence of surface states and defects (dislocations, stacking faults, and twins) in the quantum dots. The smaller crystallite size and quantum dot formation have significant effects on the high energy excitonic and low energy plasmonic absorption bands. Effective two-photon absorption coefficients measured using 100 fs laser pulses employing open-aperture Z-scan in the plasmonic region of 800 nm reveal that CuS quantum dots are better ultrafast optical limiters compared to CuS nanoparticles.

  4. Nonlinear fiber optics

    CERN Document Server

    Agrawal, Govind

    2012-01-01

    Since the 4e appeared, a fast evolution of the field has occurred. The 5e of this classic work provides an up-to-date account of the nonlinear phenomena occurring inside optical fibers, the basis of all our telecommunications infastructure as well as being used in the medical field. Reflecting the big developments in research, this new edition includes major new content: slow light effects, which offers a reduction in noise and power consumption and more ordered network traffic-stimulated Brillouin scattering; vectorial treatment of highly nonlinear fibers; and a brand new chapter o

  5. Working Beyond Moore’s Limit - Coherent Nonlinear Optical Control of Individual and Coupled Single Electron Doped Quantum Dots

    Science.gov (United States)

    2015-07-06

    Assembled InAs Quantum Dot,”, Applied Physics Letters 97, p. 113110 (2010). DOI: 10.1063/1.3487783 http://scitation.aip.org/content/ aip /journal/apl/97/11...in an InAs quantum dot. Conference on Advances in Photonics of Quantum Computing, Memory, and Communication III, JAN 27- 28, 2010 San Francisco, CA...invited Advances in Atomic, Molecular, and Optical Physics, Vol 64, Su- sanne Yelin, editor, Elsevier, Oxford (2015). 15. A. P. Burgers, J. R

  6. Quantum optics for engineers

    CERN Document Server

    Duarte, FJ

    2013-01-01

    Quantum Optics for Engineers provides a transparent and methodical introduction to quantum optics via the Dirac's bra-ket notation with an emphasis on practical applications and basic aspects of quantum mechanics such as Heisenberg's uncertainty principle and Schrodinger's equation. Self-contained and using mainly first-year calculus and algebra tools, the book:Illustrates the interferometric quantum origin of fundamental optical principles such as diffraction, refraction, and reflectionProvides a transparent introduction, via Dirac's notation, to the probability amplitude of quantum entanglem

  7. Essentials of nonlinear optics

    CERN Document Server

    Murti, Y V G S

    2014-01-01

    Current literature on Nonlinear Optics varies widely in terms of content, style, and coverage of specific topics, relative emphasis of areas and the depth of treatment. While most of these books are excellent resources for the researchers, there is a strong need for books appropriate for presenting the subject at the undergraduate or postgraduate levels in Universities. The need for such a book to serve as a textbook at the level of the bachelors and masters courses was felt by the authors while teaching courses on nonlinear optics to students of both science and engineering during the past two decades. This book has emerged from an attempt to address the requirement of presenting the subject at college level. A one-semester course covering the essentials can effectively be designed based on this.

  8. The nonlinear optical rectification and second harmonic generation in asymmetrical Gaussian potential quantum well: Effects of hydrostatic pressure, temperature and magnetic field

    Science.gov (United States)

    Liu, Xin; Zou, LiLi; Liu, Chenglin; Zhang, Zhi-Hai; Yuan, Jian-Hui

    2016-03-01

    In the present work, the effects of hydrostatic pressure, temperature, and magnetic field on the nonlinear optical rectification (OR) and second-harmonic generation (SHG) in asymmetrical Gaussian potential quantum well (QW) have been investigated theoretically. Here, the expressions for the optical properties are calculated by the compact-density-matrix approach and iterative method. Simultaneously, the energy eigenvalues and their corresponding eigenfunctions have been obtained by using the finite difference method. The energy eigenvalues and the shape of the confined potential are modulated by the hydrostatic pressure, temperature, and magnetic field. So the results of a number of numerical experiments indicate that the nonlinear OR and SHG strongly depends on the hydrostatic pressure, temperature, and magnetic field. This gives a new degree of freedom in various device applications based on the intersubband transitions of electrons.

  9. Donor impurity states and related terahertz range nonlinear optical response in GaN cylindrical quantum wires: Effects of external electric and magnetic fields

    Energy Technology Data Exchange (ETDEWEB)

    Correa, J. D. [Departamento de Ciencias Básicas, Universidad de Medellín, Medellín (Colombia); Mora-Ramos, M. E., E-mail: memora@uaem.mx [Facultad de Ciencias, Universidad Autónoma del Estado de Morelos, Av. Universidad 1001, CP 62209 Cuernavaca, Morelos (Mexico); Duque, C. A. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia)

    2014-06-07

    We report a study on the optical absorption coefficient associated to hydrogenic impurity interstate transitions in zinc-blende GaN quantum wires of cylindrical shape taking into account the effects of externally applied static electric and magnetic fields. The electron states emerge within the effective mass approximation, via the exact diagonalization of the donor-impurity Hamiltonian with parabolic confinement and external field effects. The nonlinear optical absorption is calculated using a recently derived expression for the dielectric susceptibility, obtained via a nonperturbative solution of the density-matrix Bloch equation. Our results show that this treatment eliminates not only the intensity-dependent bleaching effect but also the change in sign of the nonlinear contribution due to the combined effect of asymmetric impurity location and the applied electric field.

  10. Donor impurity states and related terahertz range nonlinear optical response in GaN cylindrical quantum wires: Effects of external electric and magnetic fields

    Science.gov (United States)

    Correa, J. D.; Mora-Ramos, M. E.; Duque, C. A.

    2014-06-01

    We report a study on the optical absorption coefficient associated to hydrogenic impurity interstate transitions in zinc-blende GaN quantum wires of cylindrical shape taking into account the effects of externally applied static electric and magnetic fields. The electron states emerge within the effective mass approximation, via the exact diagonalization of the donor-impurity Hamiltonian with parabolic confinement and external field effects. The nonlinear optical absorption is calculated using a recently derived expression for the dielectric susceptibility, obtained via a nonperturbative solution of the density-matrix Bloch equation. Our results show that this treatment eliminates not only the intensity-dependent bleaching effect but also the change in sign of the nonlinear contribution due to the combined effect of asymmetric impurity location and the applied electric field.

  11. Dielectric confinement on exciton binding energy and nonlinear optical properties in a strained Zn1-xinMgxinSe/Zn1-xoutMgxoutSe quantum well

    Institute of Scientific and Technical Information of China (English)

    J. Abraham Hudson Mark; A. John Peter

    2012-01-01

    The band offsets for a Zn1-xinMgxin Se/Zn1-xoutMgxout Se quantum well heterostructure are determined using the model solid theory.The heavy hole exciton binding energies are investigated with various Mg alloy contents.The effect of mismatch between the dielectric constants between the well and the barrier is taken into account.The dependence of the excitonic transition energies on the geometrical confinement and the Mg alloy is discussed.Non-linear optical properties are determined using the compact density matrix approach.The linear,third order non-linear optical absorption coefficient values and the refractive index changes of the exciton are calculated for different concentrations of magnesium.The results show that the occurred blue shifts of the resonant peak due to the Mg incorporation give the information about the variation of two energy levels in the quantum well width.

  12. Nonlinear absorption coefficient and optically detected electrophonon resonance in cylindrical GaAs/AlAs quantum wires with different confined phonon models

    Science.gov (United States)

    Khoa, Doan Quoc; Phuong, Le Thi Thu; Hoi, Bui Dinh

    2017-03-01

    A quantum kinetic equation for electrons interacting with confined phonons is used to investigate the nonlinear absorption of an intense electromagnetic wave by electrons in cylindrical GaAs/AlAs quantum wires. The analytic expression for absorption coefficient is calculated for three models of confined optical phonons: the dielectric continuum (DC), hydrodynamic continuum (HC), and Huang-Zhu (HZ) models. The absorption coefficient depends on the square of the electromagnetic wave amplitude. The electrophonon resonance and optically detected electrophonon resonance (ODEPR) are observed through the absorption spectrum. The full width at half maximum (the line-width) of the ODEPR peaks is obtained by a computational method. The line-width is found to increase with increasing temperature and decrease with increasing the quantum wire radius. In particular, numerical results show that the DC and HZ models lead to a similar behaviour of electron - confined phonon interaction whereas the HC model results in a quite different one, especially at small quantum wire radius. For large quantum wire radii, above mentioned phonon models have equivalent contributions to the ODEPR line-width.

  13. Terahertz Nonlinear Optics in Semiconductors

    DEFF Research Database (Denmark)

    Turchinovich, Dmitry; Hvam, Jørn Märcher; Hoffmann, Matthias C.

    2013-01-01

    We demonstrate the nonlinear optical effects – selfphase modulation and saturable absorption of a single-cycle THz pulse in a semiconductor. Resulting from THz-induced modulation of Drude plasma, these nonlinear optical effects, in particular, lead to self-shortening and nonlinear spectral...

  14. Quantum Computing: Linear Optics Implementations

    CERN Document Server

    Sundsøy, Pål

    2016-01-01

    One of the main problems that optical quantum computing has to overcome is the efficient construction of two-photon gates. Theoretically these gates can be realized using Kerr-nonlinearities, but the techniques involved are experimentally very difficult. We therefore employ linear optics with projective measurements to generate these non-linearities. The downside is that the measurement-induced nonlinearities achieved with linear optics are less versatile and the success rate can be quite low. This project is mainly the result of a literature study but also a theoretical work on the physics behind quantum optical multiports which is essential for realizing two-photon gates. By applying different postcorrection techniques we increase the probability of success in a modifed non-linear sign shift gate which is foundational for the two photon controlled-NOT gate. We prove that it's not possible to correct the states by only using a single beam splitter. We show that it might be possible to increase the probabilit...

  15. Nonlinear optical thin films

    Science.gov (United States)

    Leslie, Thomas M.

    1993-01-01

    A focused approach to development and evaluation of organic polymer films for use in optoelectronics is presented. The issues and challenges that are addressed include: (1) material synthesis, purification, and the tailoring of the material properties; (2) deposition of uniform thin films by a variety of methods; (3) characterization of material physical properties (thermal, electrical, optical, and electro-optical); and (4) device fabrication and testing. Photonic materials, devices, and systems were identified as critical technology areas by the Department of Commerce and the Department of Defense. This approach offers strong integration of basic material issues through engineering applications by the development of materials that can be exploited as the active unit in a variety of polymeric thin film devices. Improved materials were developed with unprecedented purity and stability. The absorptive properties can be tailored and controlled to provide significant improvement in propagation losses and nonlinear performance. Furthermore, the materials were incorporated into polymers that are highly compatible with fabrication and patterning processes for integrated optical devices and circuits. By simultaneously addressing the issues of materials development and characterization, keeping device design and fabrication in mind, many obstacles were overcome for implementation of these polymeric materials and devices into systems. We intend to considerably improve the upper use temperature, poling stability, and compatibility with silicon based devices. The principal device application that was targeted is a linear electro-optic modulation etalon. Organic polymers need to be properly designed and coupled with existing integrated circuit technology to create new photonic devices for optical communication, image processing, other laser applications such as harmonic generation, and eventually optical computing. The progression from microscopic sample to a suitable film

  16. Nonlinear Optical Terahertz Technology Project

    Data.gov (United States)

    National Aeronautics and Space Administration — Our approach is based on high-Q optical WGM resonators made with a nonlinear crystal. Such resonators have been demonstrated to dramatically enhance nonlinear...

  17. Second-order nonlinear optical properties in a strained InGaN/AlGaN quantum well under the intense laser field

    Science.gov (United States)

    Karimi, M. J.; Vafaei, H.

    2015-02-01

    In this work, the optical rectification and the second harmonic generation coefficients in a strained InGaN/AlGaN quantum well are studied. Impacts of the spontaneous and piezoelectric polarization fields on the potential profile are taken into account. The energy levels and wave functions are calculated using the fourth-order Runge-Kutta method and optical properties are obtained using the compact density matrix approach. Effects of intense laser field, In composition, Al composition, the well width and barrier width on the second-order nonlinear optical properties are investigated. Results reveal that the confinement potential is considerably affected by the laser field and internal electric field. Results also indicate that the resonant peaks experience a red-shift with increasing the laser field strength and barrier width. Moreover, the resonant peaks suffer a blue-shift with the increase in In and Al compositions.

  18. Focus issue introduction: nonlinear optics.

    Science.gov (United States)

    Boulanger, Benoît; Cundiff, Steven T; Gauthier, Daniel J; Karlsson, Magnus; Lu, Yan-Qing; Norwood, Robert A; Skryabin, Dmitry; Taira, Takunori

    2011-11-07

    It is now fifty years since the original observation of second harmonic generation ushered in the field of nonlinear optics, close on the heels of the invention of the laser. This feature issue celebrates this anniversary with papers that span the range from new nonlinear optical materials, through the increasingly novel methods that have been developed for phase matching, to emerging areas such as nonlinear metamaterials and plasmonic enhancement of optical properties. It is clear that the next fifty years of nonlinear optics will witness a proliferation of new applications with increasing technological impact.

  19. Creation technique and nonlinear optics of dynamic one-dimensional photonic crystals in colloidal solution of quantum dots

    Science.gov (United States)

    Smirnov, A. M.; Golinskaya, A. D.; Ezhova, K.; Kozlova, M.; Stebakova, J. V.; Valchuk, Y. V.

    2017-05-01

    One-dimensional dynamic photonic crystal was formed by a periodic spatial modulation of dielectric permittivity induced by the two ultrashort laser pulses interference in semiconductor quantum dots CdSe/ZnS (QDs) colloidal solution intersecting at angle θ. The fundamental differences of dynamic photonic crystals from static ones which determine the properties of these transient structures are the following. I. Dynamic photonic crystals lifetimes are determined by the nature of nonlinear changes of dielectric permittivity. II. The refractive index changing is determined by the intensity of the induced standing wave maxima and nonlinear susceptibility of the sample. We use the pump and probe method to create the dynamic one-dimensional photonic crystal and to analyze its features. Two focused laser beams are the pump beams, that form in the colloidal solution of quantum dots dynamic one-dimensional photonic crystal. The picosecond continuum, generated by the first harmonic of laser (1064 nm) passing through a heavy water is used as the probe beam. The self-diffraction of pumping beams on self induced dynamic one-dimensional photonic crystal provides information about spatial combining of laser beams.

  20. Nonlinear optical rectification and second-harmonic generation in a semi-parabolic quantum well under intense laser field: Effects of electric and magnetic fields

    Science.gov (United States)

    Ungan, F.; Martínez-Orozco, J. C.; Restrepo, R. L.; Mora-Ramos, M. E.; Kasapoglu, E.; Duque, C. A.

    2015-05-01

    The effects of electric and magnetic fields on the nonlinear optical rectification and second harmonic generation coefficients related with intersubband transitions in a semi-parabolic quantum well under intense laser field are theoretically studied. The energy levels and corresponding wave functions are obtained by solving the conduction band Schrödinger-like equation in the parabolic approximation and the envelope function approach. Numerical calculations are presented for a typical GaAs/Ga1-xAlxAs quantum well. The results show that both the non-resonant intense laser field and the static external fields have significant influences on the magnitude and resonant peak energy positions of the coefficients under study.

  1. Nonlinear metrology with a quantum interface

    OpenAIRE

    Napolitano, M.; Mitchell, M. W.

    2009-01-01

    We describe nonlinear quantum atom-light interfaces and nonlinear quantum metrology in the collective continuous variable formalism. We develop a nonlinear effective Hamiltonian in terms of spin and polarization collective variables and show that model Hamiltonians of interest for nonlinear quantum metrology can be produced in $^{87}$Rb ensembles. With these Hamiltonians, metrologically relevant atomic properties, e.g. the collective spin, can be measured better than the "Heisenberg limit" $\\...

  2. Quantum enhanced optical sensing

    DEFF Research Database (Denmark)

    Schäfermeier, Clemens

    The work in this thesis is embedded in the framework of quantum metrology and explores quantum effects in solid state emitters and optical sensing. Specifically, the thesis comprises studies on silicon vacancy centres in nanodiamonds, phase measurements and cavity optomechanics utilising optical...... squeezed states, and a theoretical study on quantum amplifiers. Due to its similarity to single atoms, colour centres in diamond are ideal objects for exploring and exploiting quantum effects, because they are comparably easy to produce, probe and maintain. While nitrogen vacancy centres are the most...... identified spectral diffusion as the main hindrance in extending spin coherence times. Overcoming this issue will provide a promising candidate as an emitter for quantum information. Next, the question of how squeezed states of light can improve optical sensing was addressed. For this purpose, a squeezed...

  3. Donor impurity-related linear and nonlinear intraband optical absorption coefficients in quantum ring: effects of applied electric field and hydrostatic pressure.

    Science.gov (United States)

    Barseghyan, Manuk G; Restrepo, Ricardo L; Mora-Ramos, Miguel E; Kirakosyan, Albert A; Duque, Carlos A

    2012-09-28

    : The linear and nonlinear intraband optical absorption coefficients in GaAs three-dimensional single quantum rings are investigated. Taking into account the combined effects of hydrostatic pressure and electric field, applied along the growth direction of the heterostructure, the energies of the ground and first excited states of a donor impurity have been found using the effective mass approximation and a variational method. The energies of these states are examined as functions of the dimensions of the structure, electric field, and hydrostatic pressure. We have also investigated the dependencies of the linear, nonlinear, and total optical absorption coefficients as a function of incident photon energy for several configurations of the system. It is found that the variation of distinct sizes of the structure leads to either a redshift and/or a blueshift of the resonant peaks of the intraband optical spectrum. In addition, we have found that the application of an electric field leads to a redshift, whereas the influence of hydrostatic pressure leads to a blueshift (in the case of on-ring-center donor impurity position) of the resonant peaks of the intraband optical spectrum.

  4. Nonlinear dynamics in atom optics

    Energy Technology Data Exchange (ETDEWEB)

    Chen Wenyu; Dyrting, S.; Milburn, G.J. [Queensland Univ., St. Lucia, QLD (Australia). Dept. of Physics

    1996-12-31

    In this paper theoretical work on classical and quantum nonlinear dynamics of cold atoms is reported. The basic concepts in nonlinear dynamics are reviewed and then applied to the motion of atoms in time-dependent standing waves and to the atomic bouncer. The quantum dynamics for the cases of regular and chaotic classical dynamics is described. The effect of spontaneous emission and external noise is also discussed. 104 refs., 1 tab., 21 figs.

  5. Quantum Nanoantennas for Making Nonlinear and Self-Modulatable Metasurface

    KAUST Repository

    Chen, Pai Yen

    2015-01-01

    We investigate the plasmonic nanodipole antenna with sub-microscopic nanogap. Relevant quantum conductivities, including linear and nonlinear components, are observed due to the photon-assisted quantum tunneling, realizing optical nano-radiators with enhanced amplitude and frequency modulations. © 2015 OSA.

  6. Quantum optics, what next?

    Science.gov (United States)

    Cirac, J. Ignacio; Kimble, H. Jeff

    2017-01-01

    Quantum optics is a well-established field that spans from fundamental physics to quantum information science. In the coming decade, areas including computation, communication and metrology are all likely to experience scientific and technological advances supported by this far-reaching research field.

  7. Nonlinear Optics: Principles and Applications

    DEFF Research Database (Denmark)

    Rottwitt, Karsten; Tidemand-Lichtenberg, Peter

    As nonlinear optics further develops as a field of research in electromagnetic wave propagation, its state-of-the-art technologies will continue to strongly impact real-world applications in a variety of fields useful to the practicing scientist and engineer. From basic principles to examples...... of applications, Nonlinear Optics: Principles and Applications effectively bridges physics and mathematics with relevant applied material for real-world use. The book progresses naturally from fundamental aspects to illustrative examples, and presents a strong theoretical foundation that equips the reader...... and matter, this text focuses on the physical understanding of nonlinear optics, and explores optical material response functions in the time and frequency domain....

  8. Field guide to nonlinear optics

    CERN Document Server

    Powers, Peter E

    2013-01-01

    Optomechanics is a field of mechanics that addresses the specific design challenges associated with optical systems. This [i]Field Guide [/i]describes how to mount optical components, as well as how to analyze a given design. It is intended for practicing optical and mechanical engineers whose work requires knowledge in both optics and mechanics. This Field Guide is designed for those looking for a condensed and concise source of key concepts, equations, and techniques for nonlinear optics. Topics covered include technologically important effects, recent developments in nonlinear optics

  9. Optical quantum computing.

    Science.gov (United States)

    O'Brien, Jeremy L

    2007-12-07

    In 2001, all-optical quantum computing became feasible with the discovery that scalable quantum computing is possible using only single-photon sources, linear optical elements, and single-photon detectors. Although it was in principle scalable, the massive resource overhead made the scheme practically daunting. However, several simplifications were followed by proof-of-principle demonstrations, and recent approaches based on cluster states or error encoding have dramatically reduced this worrying resource overhead, making an all-optical architecture a serious contender for the ultimate goal of a large-scale quantum computer. Key challenges will be the realization of high-efficiency sources of indistinguishable single photons, low-loss, scalable optical circuits, high-efficiency single-photon detectors, and low-loss interfacing of these components.

  10. Quantum Dynamics of Nonlinear Cavity Systems

    OpenAIRE

    Nation, Paul D.

    2010-01-01

    We investigate the quantum dynamics of three different configurations of nonlinear cavity systems. To begin, we carry out a quantum analysis of a dc superconducting quantum interference device (SQUID) mechanical displacement detector comprised of a SQUID with a mechanically compliant loop segment. The SQUID is approximated by a nonlinear current-dependent inductor, inducing a flux tunable nonlinear Duffing term in the cavity equation of motion. Expressions are derived for the detector signal ...

  11. Chiral quantum optics.

    Science.gov (United States)

    Lodahl, Peter; Mahmoodian, Sahand; Stobbe, Søren; Rauschenbeutel, Arno; Schneeweiss, Philipp; Volz, Jürgen; Pichler, Hannes; Zoller, Peter

    2017-01-25

    Advanced photonic nanostructures are currently revolutionizing the optics and photonics that underpin applications ranging from light technology to quantum-information processing. The strong light confinement in these structures can lock the local polarization of the light to its propagation direction, leading to propagation-direction-dependent emission, scattering and absorption of photons by quantum emitters. The possibility of such a propagation-direction-dependent, or chiral, light-matter interaction is not accounted for in standard quantum optics and its recent discovery brought about the research field of chiral quantum optics. The latter offers fundamentally new functionalities and applications: it enables the assembly of non-reciprocal single-photon devices that can be operated in a quantum superposition of two or more of their operational states and the realization of deterministic spin-photon interfaces. Moreover, engineered directional photonic reservoirs could lead to the development of complex quantum networks that, for example, could simulate novel classes of quantum many-body systems.

  12. Nonlinear optics principles and applications

    CERN Document Server

    Li, Chunfei

    2017-01-01

    This book reflects the latest advances in nonlinear optics. Besides the simple, strict mathematical deduction, it also discusses the experimental verification and possible future applications, such as the all-optical switches. It consistently uses the practical unit system throughout. It employs simple physical images, such as "light waves" and "photons" to systematically explain the main principles of nonlinear optical effects. It uses the first-order nonlinear wave equation in frequency domain under the condition of “slowly varying amplitude approximation" and the classical model of the interaction between the light and electric dipole. At the same time, it also uses the rate equations based on the energy-level transition of particle systems excited by photons and the energy and momentum conservation principles to explain the nonlinear optical phenomenon. The book is intended for researchers, engineers and graduate students in the field of the optics, optoelectronics, fiber communication, information tech...

  13. Nonlinear Michelson interferometer for improved quantum metrology

    Science.gov (United States)

    Luis, Alfredo; Rivas, Ángel

    2015-08-01

    We examine quantum detection via a Michelson interferometer embedded in a gas with Kerr nonlinearity. This nonlinear interferometer is illuminated by pulses of classical light. This strategy combines the robustness against practical imperfections of classical light with the improvement provided by nonlinear processes. Regarding ultimate quantum limits, we stress that, as a difference with linear schemes, the nonlinearity introduces pulse duration as a new variable into play along with the energy resources.

  14. Nonlinear Michelson interferometer for improved quantum metrology

    OpenAIRE

    Luis Aina, Alfredo; Rivas Vargas, Ángel

    2015-01-01

    We examine quantum detection via a Michelson interferometer embedded in a gas with Kerr nonlinearity. This nonlinear interferometer is illuminated by pulses of classical light. This strategy combines the robustness against practical imperfections of classical light with the improvement provided by nonlinear processes. Regarding ultimate quantum limits, we stress that, as a difference with linear schemes, the nonlinearity introduces pulse duration as a new variable into play along with the ene...

  15. Optically nonlinear materials

    CERN Document Server

    Whittam, A J

    2001-01-01

    susceptibility from 26 pm/V (same film without octadecanoic acid) to 40 pm/V. This increase in the second-order susceptibility occurred even though the amount of NLO-active dye was effectively diluted by the addition of the inactive octadecanoic acid. The wavelength of the absorption maximum ranged from 346-440 nm and there was direct correlation between the susceptibilities and the transparency of the films at the harmonic wavelength. Hemicyanine dyes were synthesised, with the general formulae: - (a) C sub 1 sub 8 H sub 3 sub 7 -A sup + -[CH=CH-C sub 6 H sub 4] sub x -N(CH sub 3) sub 2 I (b) C sub 1 sub 8 H sub 3 sub 7 -A sup + -[CH=CH] sub y -C sub 6 H sub 4 -N(CH sub 3) sub 2 I where A sup + is a pyridinium or isoquinolinium acceptor, and x = 1 or 2, and y = 1 or 2. The optically nonlinear dyes were investigated via the Langmuir-Blodgett (LB) technique. The dyes all produced isotherm data, with molecular areas of 22-60 A sup 2 per molecule, which are consistent with the cross-sectional areas of the chromo...

  16. Advances in chemical physics modern nonlinear optics, pt.1

    CERN Document Server

    Rice, Stuart A

    2009-01-01

    Partial table of contents: Hyper-Rayleigh and Hyper-Raman Rotational and Vibrational Spectroscopy (T. Bancewicz & Z. Ożgo). Polarization Properties of Hyper-Rayleigh and Hyper-Raman Scatterings (M. Kozierowski). Fast Molecular Reorientation in Liquid Crystals Probed by Nonlinear Optics (J. Lalanne, et al.). Nonlinear Propagation of Laser Light of Different Polarizations (G. Rivoire). Nonlinear Magneto-Optics of Magnetically Ordered Crystals (R. Zawodny). Dynamical Questions in Quantum Optics (A. Shumovsky). Quantum Resonance Fluorescence from Mutually Correlated Atoms (Z. Fi

  17. Synthesis, an experimental and quantum chemical computational study of a new nonlinear optical material: 2-picolinium hydrogensquarate.

    Science.gov (United States)

    Korkmaz, Ufuk; Bulut, Ahmet

    2014-09-15

    The experimental and theoretical investigation results of a novel organic non-linear optical (NLO) organic squarate salt of 2-Picolinium hydrogensquarate (1), C6H8N+·C4HO4-, were reported in this study. The space group of the title compound was found in the monoclinic C2/c space group. It was found that the asymmetric unit consists of one monohydrogen squarate anion together with mono protonated 2-Picolinium, forming the (1) salt. The X-ray analysis clearly indicated that the crystal packing has shown the hydrogen bonding ring pattern of D2(2)(10) (α-dimer) through NH⋯O interactions. The hydrogensquarate anions form α-dimer, while 2-Picolinium molecule interacts through NH⋯O and CH⋯O with the hydrogensquarate anion. The structural and vibrational properties of the compound were also studied by computational methods of ab initio performed on the compound at DFT/B3LYP/6-31++G(d,p) (2) and HF/6-31++G(d,p) (3) level of theory. The calculation results on the basis of two models for both the optimized molecular structure and vibrational properties for the 1 obtained are presented and compared with the X-ray analysis result. On the other the molecular electrostatic potential (MEP), electronic absorption spectra, frontier molecular orbitals (FMOs), conformational flexibility and non-linear optical properties (NLO) of the title compound were also studied at the 2 level and the results are reported. In order to evaluate the suitability for NLO applications thermal analysis (TG, DTA and DTG) data of 1 were also obtained.

  18. Momentum Transfer Studies and Studies of Linear and Nonlinear Optical Properties of Metal Colloids and Semiconductor Quantum Dots

    Science.gov (United States)

    Collins, W. E.; Burger, A.; Dyer, K.; George, M.; Henderson, D.; Morgan, S.; Mu, R.; Shi, D.; Conner, D; Thompson, E.; Collins, L.; Curry, L.; Mattox, S.; Williams, G.

    1996-01-01

    Phase 1 of this work involved design work on a momentum transfer device. The progress on design and testing will be presented. Phase 2 involved the systematic study of the MPD thruster for dual uses. Though it was designed as a thruster for space vehicles, the characteristics of the plasma make it an excellent candidate for industrial applications. This project sought to characterize the system for use in materials processing and characterization. The surface modification on ZnCdTe, CdTe, and ZnTe will be presented. Phase 3 involved metal colloids and semiconductor quantum dots. One aspect of this project involves a collaborative effort with the Solid State Division of ORNL. The thrust behind this research is to develop ion implantation for synthesizing novel materials (quantum dots wires and wells, and metal colloids) for applications in all optical switching devices, up conversion, and the synthesis of novel refractory materials. The ions of interest are Au, Ag, Cd, Se, In, P, Sb, Ga, and As. The specific materials of interest are: CdSe, CdTe, InAs, GaAs, InP, GaP, InSb, GaSb, and InGaAs. A second aspect of this research program involves using porous glass (25-200 A) for fabricating materials of finite size. The results of some of this work will also be reported.

  19. Momentum Transfer Studies and Studies of Linear and Nonlinear Optical Properties of Metal Colloids and Semiconductor Quantum Dots

    Science.gov (United States)

    Collins, W. E.; Burger, A.; Dyer, K.; George, M.; Henderson, D.; Morgan, S.; Mu, R.; Shi, D.; Conner, D; Thompson, E.; hide

    1996-01-01

    Phase 1 of this work involved design work on a momentum transfer device. The progress on design and testing will be presented. Phase 2 involved the systematic study of the MPD thruster for dual uses. Though it was designed as a thruster for space vehicles, the characteristics of the plasma make it an excellent candidate for industrial applications. This project sought to characterize the system for use in materials processing and characterization. The surface modification on ZnCdTe, CdTe, and ZnTe will be presented. Phase 3 involved metal colloids and semiconductor quantum dots. One aspect of this project involves a collaborative effort with the Solid State Division of ORNL. The thrust behind this research is to develop ion implantation for synthesizing novel materials (quantum dots wires and wells, and metal colloids) for applications in all optical switching devices, up conversion, and the synthesis of novel refractory materials. The ions of interest are Au, Ag, Cd, Se, In, P, Sb, Ga, and As. The specific materials of interest are: CdSe, CdTe, InAs, GaAs, InP, GaP, InSb, GaSb, and InGaAs. A second aspect of this research program involves using porous glass (25-200 A) for fabricating materials of finite size. The results of some of this work will also be reported.

  20. Concepts of quantum optics

    CERN Document Server

    Knight, P L

    1983-01-01

    Concepts of Quantum Optics is a coherent and sequential coverage of some real insight into quantum physics. This book is divided into six chapters, and begins with an overview of the principles and concepts of radiation and quanta, with an emphasis on the significance of the Maxwell's electromagnetic theory of light. The next chapter describes first the properties of the radiation field in a bounded cavity, showing how each cavity field mode has the characteristics of a simple harmonic oscillator and how each can be quantized using known results for the quantum harmonic oscillator. This chapte

  1. Nonlinear optics: the next decade.

    Science.gov (United States)

    Kivshar, Yuri S

    2008-12-22

    This paper concludes the Focus Serial assembled of invited papers in key areas of nonlinear optics (Editors: J.M. Dudley and R.W. Boyd), and it discusses new directions for future research in this field.

  2. Rotational Doppler effect in nonlinear optics

    Science.gov (United States)

    Li, Guixin; Zentgraf, Thomas; Zhang, Shuang

    2016-08-01

    The translational Doppler effect of electromagnetic and sound waves has been successfully applied in measurements of the speed and direction of vehicles, astronomical objects and blood flow in human bodies, and for the Global Positioning System. The Doppler effect plays a key role for some important quantum phenomena such as the broadened emission spectra of atoms and has benefited cooling and trapping of atoms with laser light. Despite numerous successful applications of the translational Doppler effect, it fails to measure the rotation frequency of a spinning object when the probing wave propagates along its rotation axis. This constraint was circumvented by deploying the angular momentum of electromagnetic waves--the so-called rotational Doppler effect. Here, we report on the demonstration of rotational Doppler shift in nonlinear optics. The Doppler frequency shift is determined for the second harmonic generation of a circularly polarized beam passing through a spinning nonlinear optical crystal with three-fold rotational symmetry. We find that the second harmonic generation signal with circular polarization opposite to that of the fundamental beam experiences a Doppler shift of three times the rotation frequency of the optical crystal. This demonstration is of fundamental significance in nonlinear optics, as it provides us with insight into the interaction of light with moving media in the nonlinear optical regime.

  3. Oscillating solitons in nonlinear optics

    Indian Academy of Sciences (India)

    Lin Xiao-Gang; Liu Wen-Jun; Lei Ming

    2016-03-01

    Oscillating solitons are obtained in nonlinear optics. Analytical study of the variable coefficient nonlinear Schrödinger equation, which is used to describe the soliton propagation in those systems, is carried out using the Hirota’s bilinear method. The bilinear forms and analytic soliton solutions are derived, and the relevant properties and features of oscillating solitons are illustrated. Oscillating solitons are controlled by the reciprocal of the group velocity and Kerr nonlinearity. Results of this paper will be valuable to the study of dispersion-managed optical communication system and mode-locked fibre lasers.

  4. Quantum optics with semiconductor nanostructures

    CERN Document Server

    Jahnke, Frank

    2012-01-01

    A guide to the theory, application and potential of semiconductor nanostructures in the exploration of quantum optics. It offers an overview of resonance fluorescence emission.$bAn understanding of the interaction between light and matter on a quantum level is of fundamental interest and has many applications in optical technologies. The quantum nature of the interaction has recently attracted great attention for applications of semiconductor nanostructures in quantum information processing. Quantum optics with semiconductor nanostructures is a key guide to the theory, experimental realisation, and future potential of semiconductor nanostructures in the exploration of quantum optics. Part one provides a comprehensive overview of single quantum dot systems, beginning with a look at resonance fluorescence emission. Quantum optics with single quantum dots in photonic crystal and micro cavities are explored in detail, before part two goes on to review nanolasers with quantum dot emitters. Light-matter interaction...

  5. Nonlinear optics and organic materials

    Energy Technology Data Exchange (ETDEWEB)

    Shen, Y.R.

    1994-07-01

    We shall consider an interesting topic relating nonlinear optics and organic materials: how nonlinear optics can be used to study organic materials. One of the main differences between linear and nonlinear responses of a medium to incoming radiation is in their symmetries. It leads to the possibility that some properties of the medium could be more sensitively probed by nonlinear, rather than linear, optical means, or vise versa. A well-known example is that some vibrational modes of a medium could be Raman-active but infrared-inactive, and would be more readily observed by Raman scattering, which is a two-photon transition process. In this paper, we shall discuss, with the help of three examples, how we can use second harmonic generation (SHG) and sum frequency generation (SFG) to obtain unique information about a material. We shall focus on thin films, surfaces, and interfaces.

  6. Nonlinear Optics and Turbulence

    Science.gov (United States)

    1992-10-01

    currently at Queen Mary College, London Patrick Dunne, (Ph.D., 1987, M.I.T., Hydrodynamic Stability, Nonlinear Waves), 1987-1988. Alecsander Dyachenko...U I I I U I I 3 9 3 V. BIOGRAPHIES A. FACULTY BRUCE BAYLY, 31, Ph.D. 1986, Princeton University. Postdoctoral visiting member 1986-88 at Courant...Caputo, A. C. Newell, and M. Shelley , "Nonlinear Wave Propagation Through a Random Medium and Soliton Tunneling", Integrable Systems and

  7. Optoelectronic and nonlinear optical processes in low dimensional semiconductors

    Indian Academy of Sciences (India)

    B P Singh

    2006-11-01

    Spatial confinement of quantum excitations on their characteristic wavelength scale in low dimensional materials offers unique possibilities to engineer the electronic structure and thereby control their physical properties by way of simple manipulation of geometrical parameters. This has led to an overwhelming interest in quasi-zero dimensional semiconductors or quantum dots as tunable materials for multitude of exciting applications in optoelectronic and nonlinear optical devices and quantum information processing. Large nonlinear optical response and high luminescence quantum yield expected in these systems is a consequence of huge enhancement of transition probabilities ensuing from quantum confinement. High quantum efficiency of photoluminescence, however, is not usually realized in the case of bare semiconductor nanoparticles owing to the presence of surface states. In this talk, I will focus on the role of quantum confinement and surface states in ascertaining nonlinear optical and optoelectronic properties of II–VI semiconductor quantum dots and their nanocomposites. I will also discuss the influence of nonlinear optical processes on their optoelectronic characteristics.

  8. Simulation of an optomechanical quantum memory in the nonlinear regime

    Science.gov (United States)

    Teh, R. Y.; Kiesewetter, S.; Reid, M. D.; Drummond, P. D.

    2017-07-01

    Optomechanical systems cooled to the quantum level provide a promising mechanism for a high-fidelity quantum memory that is faithful to a given temporal mode structure, and can be recovered synchronously. We carry out full, probabilistic quantum simulation of a quantum optomechanical memory, including nonlinear effects that are usually ignored. This is achieved using both the approximate truncated Wigner and the exact positive P phase-space representations. By considering the nonlinear quantum optomechanical Hamiltonian, our simulations allow us to probe the regime where the linearization approximation fails to hold. We show evidence for large spectral overlap between the quantum signal and the transfer field in typical optomechanical quantum memory experiments. Methods for eliminating this overlap to accurately recover the quantum signal are discussed. This allows us to give a complete model for the quantum storage of a coherent state. We treat the mode matching that is necessary to accurately retrieve the stored quantum state, by including the internal dynamics of the mechanical system as well as the optical system. We also include the finite switching time of the control transfer field. The fidelity for the storage of a coherent state is computed numerically using currently realistic experimental parameters in the electromechanical case. We find the expected fidelity is lower than required to demonstrate true quantum state transfers. Significant improvements in the quality factor of the cavity and mechanical systems will, however, increase the fidelity beyond the quantum threshold.

  9. Asymmetric GaAs n-type double δ-doped quantum wells as a source of intersubband-related nonlinear optical response: Effects of an applied electric field

    Energy Technology Data Exchange (ETDEWEB)

    Rodríguez-Magdaleno, K.A.; Martínez-Orozco, J.C.; Rodríguez-Vargas, I. [Unidad Académica de Física, Universidad Autónoma de Zacatecas, Calz. Solidaridad Esq. Paseo a La Bufa S/N. C.P. 98060 Zacatecas (Mexico); Mora-Ramos, M.E. [Facultad de Ciencias, Universidad Autónoma del Estado de Morelos, Av. Universidad 1001, CP 62209 Cuernavaca, Morelos (Mexico); Física Teórica y Aplicada, Escuela de Ingeniería de Antioquia, AA 7516 Medellín (Colombia); Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia); Duque, C.A., E-mail: cduque@fisica.udea.edu.co [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia)

    2014-03-15

    In this work, the conduction band electron states and the associated intersubband-related linear and nonlinear optical absorption coefficient and relative refractive index change are calculated for an asymmetric double n-type δ-doped quantum well in a GaAs-matrix. The effects of an external applied static electric field are included. Values of the two-dimensional impurities density (N{sub 2d}) of each single δ-doped quantum well are taken to vary within the range of 1.0×10{sup 12} to 7.0×10{sup 12} cm{sup −2}, consistent with the experimental data growth regime. The optical responses are reported as a function of the δ-doped impurities density and the applied electric field. It is shown that single electron states and the related optical quantities are significantly affected by the structural asymmetry of the double δ-doped quantum well system. In addition, a brief comparison with the free-carrier-related optical response is presented. -- Highlights: • Nonlinear optics in asymmetric double n-type δ-doped quantum well in a GaAs-matrix. • The system is considered under external applied electric field in growth direction. • The 2D impurity density is consistent with the experimental data growth regime. • The optical quantities are significantly affected by the structural asymmetry of the system.

  10. Nonlinear fiber applications for ultrafast all-optical signal processing

    Science.gov (United States)

    Kravtsov, Konstantin

    In the present dissertation different aspects of all-optical signal processing, enabled by the use of nonlinear fibers, are studied. In particular, we focus on applications of a novel heavily GeO2-doped (HD) nonlinear fiber, that appears to be superior to many other types of nonlinear fibers because of its high nonlinearity and suitability for the use in nonlinear optical loop mirrors (NOLMs). Different functions, such as all-optical switching, thresholding, and wavelength conversion, are demonstrated with the HD fibers in the NOLM configuration. These basic functions are later used for realization of ultrafast time-domain demultiplexers, clock recovery, detectors of short pulses in stealth communications, and primitive elements for analog computations. Another important technology that benefits from the use of nonlinear fiber-based signal processing is optical code-division multiple access (CDMA). It is shown in both theory and experiment that all-optical thresholding is a unique way of improving existing detection methods for optical CDMA. Also, it is the way of implementation of true asynchronous optical spread-spectrum networks, which allows full realization of optical CDMA potential. Some aspects of quantum signal processing and manipulation of quantum states are also studied in this work. It is shown that propagation and collisions of Thirring solitons lead to a substantial squeezing of quantum states, which may find applications for generation of squeezed light.

  11. Nonlinear pulse propagation in InAs/InP quantum-dot optical amplifiers: Rabi-oscillations in the presence of non-resonant nonlinearities

    CERN Document Server

    Karni, Ouri; Eisenstein, Gad; Reithmaier, Johann Peter

    2014-01-01

    We study the interplay between coherent light-matter interactions and non-resonant pulse propagation effects when ultra-short pulses propagate in room-temperature quantum-dot (QD) semiconductor optical amplifiers (SOAs). The signatures observed on a pulse envelope after propagating in a transparent SOA, when coherent Rabi-oscillations are absent, highlight the contribution of two-photon absorption (TPA), and its accompanying Kerr-like effect, as well as of linear dispersion, to the modification of the pulse complex electric field profile. These effects are incorporated into our previously developed finite-difference time-domain comprehensive model that describes the interaction between the pulses and the QD SOA. The present, generalized, model is used to investigate the combined effect of coherent and non-resonant phenomena in the gain and absorption regimes of the QD SOA. It confirms that in the QD SOA we examined, linear dispersion in the presence of the Kerr-like effect causes pulse compression, which coun...

  12. Measurement-Induced Strong Kerr Nonlinearity for Weak Quantum States of Light

    Science.gov (United States)

    Costanzo, Luca S.; Coelho, Antonio S.; Biagi, Nicola; Fiurášek, Jaromír; Bellini, Marco; Zavatta, Alessandro

    2017-07-01

    Strong nonlinearity at the single photon level represents a crucial enabling tool for optical quantum technologies. Here we report on experimental implementation of a strong Kerr nonlinearity by measurement-induced quantum operations on weak quantum states of light. Our scheme coherently combines two sequences of single photon addition and subtraction to induce a nonlinear phase shift at the single photon level. We probe the induced nonlinearity with weak coherent states and characterize the output non-Gaussian states with quantum state tomography. The strong nonlinearity is clearly witnessed as a change of sign of specific off-diagonal density matrix elements in the Fock basis.

  13. New nonlinear optical materials based on ferrofluids

    Energy Technology Data Exchange (ETDEWEB)

    Huang, J P [Department of Physics, Fudan University, Shanghai 200433 (China); Max Planck Institute for Polymer Research, Ackermannweg 10, 55128 Mainz (Germany); Institute of Theoretical Physics, Chinese University of Hong Kong, Shatin, NT, Hong Kong (China); Yu, K W [Department of Physics, Chinese University of Hong Kong, Shatin, NT, Hong Kong (China); Institute of Theoretical Physics, Chinese University of Hong Kong, Shatin, NT, Hong Kong (China)

    2006-01-01

    We exploit theoretically a new class of magneto-controlled nonlinear optical material based on ferrofluids in which ferromagnetic nanoparticles are coated with a nonmagnetic metallic nonlinear shell. Such an optical material can have anisotropic nonlinear optical properties and a giant enhancement of nonlinearity, as well as an attractive figure of merit.

  14. Terahertz semiconductor nonlinear optics

    DEFF Research Database (Denmark)

    Turchinovich, Dmitry; Hvam, Jørn Märcher; Hoffmann, Matthias

    2013-01-01

    nonlinearity in doped semiconductors originates from the near-instantaneous heating of free electrons in the ponderomotive potential created by electric field of the THz pulse, leading to ultrafast increase of electron effective mass by intervalley scattering. Modification of effective mass in turn leads...

  15. Linear and nonlinear optical absorption coefficients in GaAs/Ga{sub 1-x}Al{sub x}As concentric double quantum rings: Effects of hydrostatic pressure and aluminum concentration

    Energy Technology Data Exchange (ETDEWEB)

    Baghramyan, H.M. [Department of Solid State Physics, Yerevan State University, Al. Manookian 1, 0025 Yerevan (Armenia); Barseghyan, M.G., E-mail: mbarsegh@ysu.am [Department of Solid State Physics, Yerevan State University, Al. Manookian 1, 0025 Yerevan (Armenia); Kirakosyan, A.A. [Department of Solid State Physics, Yerevan State University, Al. Manookian 1, 0025 Yerevan (Armenia); Restrepo, R.L. [Escuela de Ingenieria de Antioquia, AA 7516 Medellin (Colombia); Duque, C.A. [Instituto de Fisica, Universidad de Antioquia, AA 1226 Medellin (Colombia)

    2013-02-15

    The linear and nonlinear intra-band optical absorption coefficients in GaAs/Ga{sub 1-x}Al{sub x}As two-dimensional concentric double quantum rings are investigated. Taking into account the combined effects of hydrostatic pressure and aluminum concentration the energies of the ground (n=1,l=0) and the first excited state (n=2,l=1) have been found using the effective mass approximation and the transfer matrix formalism. The energies of these states and the corresponding threshold energy of the intra-band optical transitions are examined as a function of hydrostatic pressure and aluminum concentration for different sizes of the structure. We also investigated the dependencies of the linear, nonlinear, and total optical absorption coefficients as functions of the incident photon energy for different values of hydrostatic pressure, aluminum concentration, sizes of the structure, and incident optical intensity. Its is found that the effects of the hydrostatic pressure and the aluminum concentration lead to a shifting of the resonant peaks of the intra-band optical spectrum. - Highlights: Black-Right-Pointing-Pointer Linear and nonlinear intra-band absorption in quantum rings. Black-Right-Pointing-Pointer Threshold energy strongly depends on the hydrostatic pressure. Black-Right-Pointing-Pointer Threshold energy strongly depends on the stoichiometry and sizes of structure. Black-Right-Pointing-Pointer Optical absorption is affected by the incident optical intensity.

  16. Resource Letter NO-1: Nonlinear Optics

    Science.gov (United States)

    Garmire, Elsa

    2011-03-01

    This Resource Letter provides a guide to the literature on nonlinear optics. Books, journals, and websites are introduced that cover the general subject. Journal articles and websites are cited covering the following topics: second-order nonlinearities in transparent media including second-harmonic generation and optical parametric oscillation, third-order and higher nonlinearities, nonlinear refractive index, absorptive nonlinearities such as saturable absorption and multiphoton absorption, and scattering nonlinearities such as stimulated Raman scattering and stimulated Brillouin scattering. Steady-state and transient phenomena, fiber optics, solitons, nonlinear wave mixing, optical phase conjugation, nonlinear spectroscopy, and multiphoton microscopy are all outlined.

  17. Chiral Quantum Optics

    CERN Document Server

    Lodahl, Peter; Stobbe, Søren; Schneeweiss, Philipp; Volz, Jürgen; Rauschenbeutel, Arno; Pichler, Hannes; Zoller, Peter

    2016-01-01

    At the most fundamental level, the interaction between light and matter is manifested by the emission and absorption of single photons by single quantum emitters. Controlling light--matter interaction is the basis for diverse applications ranging from light technology to quantum--information processing. Many of these applications are nowadays based on photonic nanostructures strongly benefitting from their scalability and integrability. The confinement of light in such nanostructures imposes an inherent link between the local polarization and propagation direction of light. This leads to {\\em chiral light--matter interaction}, i.e., the emission and absorption of photons depend on the propagation direction and local polarization of light as well as the polarization of the emitter transition. The burgeoning research field of {\\em chiral quantum optics} offers fundamentally new functionalities and applications both for single emitters and ensembles thereof. For instance, a chiral light--matter interface enables...

  18. Nonlinear wave interactions in quantum magnetoplasmas

    CERN Document Server

    Shukla, P K; Marklund, M; Stenflo, L

    2006-01-01

    Nonlinear interactions involving electrostatic upper-hybrid (UH), ion-cyclotron (IC), lower-hybrid (LH), and Alfven waves in quantum magnetoplasmas are considered. For this purpose, the quantum hydrodynamical equations are used to derive the governing equations for nonlinearly coupled UH, IC, LH, and Alfven waves. The equations are then Fourier analyzed to obtain nonlinear dispersion relations, which admit both decay and modulational instabilities of the UH waves at quantum scales. The growth rates of the instabilities are presented. They can be useful in applications of our work to diagnostics in laboratory and astrophysical settings.

  19. Dynamic optical hysteresis in the quantum regime

    CERN Document Server

    Rodriguez, S R K; Storme, F; Sagnes, I; Gratiet, L Le; Galopin, E; Lemaitre, A; Amo, A; Ciuti, C; Bloch, J

    2016-01-01

    For more than 40 years, optical bistability --- the existence of two stable states with different photon numbers for the same driving conditions --- has been experimentally reported. Surprisingly, the quantum theory of a single-mode nonlinear cavity always predicts a unique steady state, i.e. no bistability. To reconcile this apparent contradiction, a tunneling time for bistability has been introduced. This is a timescale over which quantum fluctuations trigger transitions between classically stable states, and which can be astronomically longer than the measurement. While quantum fluctuations ultimately forbid the static hysteresis associated with bistability, it was recently predicted that optical hysteresis should emerge dynamically for finite sweep rates of the driving intensity. This dynamic hysteresis is expected to exhibit a double power-law behavior defining a classical-to-quantum crossover. Here, by measuring the dynamic optical hysteresis of a semiconductor microcavity for various sweep rates of the...

  20. Quantum optical rotatory dispersion

    Science.gov (United States)

    Tischler, Nora; Krenn, Mario; Fickler, Robert; Vidal, Xavier; Zeilinger, Anton; Molina-Terriza, Gabriel

    2016-01-01

    The phenomenon of molecular optical activity manifests itself as the rotation of the plane of linear polarization when light passes through chiral media. Measurements of optical activity and its wavelength dependence, that is, optical rotatory dispersion, can reveal information about intricate properties of molecules, such as the three-dimensional arrangement of atoms comprising a molecule. Given a limited probe power, quantum metrology offers the possibility of outperforming classical measurements. This has particular appeal when samples may be damaged by high power, which is a potential concern for chiroptical studies. We present the first experiment in which multiwavelength polarization-entangled photon pairs are used to measure the optical activity and optical rotatory dispersion exhibited by a solution of chiral molecules. Our work paves the way for quantum-enhanced measurements of chirality, with potential applications in chemistry, biology, materials science, and the pharmaceutical industry. The scheme that we use for probing wavelength dependence not only allows one to surpass the information extracted per photon in a classical measurement but also can be used for more general differential measurements. PMID:27713928

  1. Nonlinear Optical Response of Conjugated Polymer to Electric Field

    Institute of Scientific and Technical Information of China (English)

    ZHOU Yu-fang; ZHUANG De-xin; CUI Bin

    2005-01-01

    The organic π-conjugated polymers are of major interest materials for the use in electro-optical and nonlinear optical devices. In this work, for a selected polyacetylene chain, the optical absorption spectra in UV/Vis regime as well as the linear polarizabilitiy and nonlinear hyperpolarizability are calculated by using quantum chemical ab initio and semiempirical methods. The relationship of its optical property to electric field is obtained. Some physical mechanism of electric field effect on molecular optical property is discussed by means of electron distribution and intramolecular charge transfer.

  2. Preparation and third-order nonlinear optical properties of self-organized complex oxide Ce: BaTiO3 quantum dots

    Institute of Scientific and Technical Information of China (English)

    师文生; 陈正豪; 刘宁宁; 吕惠宾; 周岳亮; 崔大复; 杨国桢

    2000-01-01

    Pulsed laser ablation epitaxial Strancky-Krastanow growth of self-organized complex oxide Ce:BaTiO3 quantum dots on MgO(100) substrates is demonstrated. Atomic force microscopy and X-ray diffraction are used to observe the structure and the growth process of the self-organized complex oxide quantum dots. The average dimension, height, and the density of self-organized complex oxide Ce:BaTiO3 quantum dots are given. The nonlinear refractive indexes of the wetting layer and the self-organized ordered quantum dots are determined by the single beam Z-scan method. The mechanisms of the nonlinear effect enhancement for these low-dimensional structure are discussed.

  3. Preparation and third-order nonlinear optical properties of self-organized complex oxide Ce:BaTiO3 quantum dots

    Institute of Scientific and Technical Information of China (English)

    2000-01-01

    Pulsed laser ablation epitaxial Strancky-Krastanow growth of self-organized complex oxide Ce:BaTiO3 quantum dots on MgO(100) substrates is demonstrated.Atomic force microscopy and X-ray diffraction are used to observe the structure and the growth process of the self-organized complex oxide quantum dots.The average dimension,height,and the density of self-organized complex oxide Ce:BaTiO3 quantum dots are given.The nonlinear refractive indexes of the wetting layer and the self-organized ordered quantum dots are determined by the single beam Z-scan method.The mechanisms of the nonlinear effect enhancement for these low-dimensional structure are discussed.

  4. Nonlinear Optics of Hexaphenyl Nanofibers

    DEFF Research Database (Denmark)

    Balzer, Frank; Al-Shamery, Katharina; Neuendorf, Rolf

    2003-01-01

    measurements reveal that the nonlinear optical transition dipole moment is oriented with an angle of 75° with respect to the needles long axes. The absolute value of the macroscopic second-order susceptibility, averaged over a size distribution of p-6P nanoaggregates, is estimated to be of the order of 6...

  5. Nonlinear Dynamics In Quantum Physics -- Quantum Chaos and Quantum Instantons

    OpenAIRE

    Kröger, H.

    2003-01-01

    We discuss the recently proposed quantum action - its interpretation, its motivation, its mathematical properties and its use in physics: quantum mechanical tunneling, quantum instantons and quantum chaos.

  6. Nonlinear Dynamics In Quantum Physics -- Quantum Chaos and Quantum Instantons

    OpenAIRE

    Kröger, H.

    2003-01-01

    We discuss the recently proposed quantum action - its interpretation, its motivation, its mathematical properties and its use in physics: quantum mechanical tunneling, quantum instantons and quantum chaos.

  7. Quantum theory of the optical and electronic properties of semiconductors

    CERN Document Server

    Haug, Hartmut

    2009-01-01

    This invaluable textbook presents the basic elements needed to understand and research into semiconductor physics. It deals with elementary excitations in bulk and low-dimensional semiconductors, including quantum wells, quantum wires and quantum dots. The basic principles underlying optical nonlinearities are developed, including excitonic and many-body plasma effects. Fundamentals of optical bistability, semiconductor lasers, femtosecond excitation, the optical Stark effect, the semiconductor photon echo, magneto-optic effects, as well as bulk and quantum-confined Franz-Keldysh effects, are covered. The material is presented in sufficient detail for graduate students and researchers with a general background in quantum mechanics.This fifth edition includes an additional chapter on 'Quantum Optical Effects' where the theory of quantum optical effects in semiconductors is detailed. Besides deriving the 'semiconductor luminescence equations' and the expression for the stationary luminescence spectrum, the resu...

  8. Exciton-related nonlinear optical response and photoluminescence in dilute nitrogen In{sub x}Ga{sub 1−x}N{sub y}As{sub 1−y}/GaAs cylindrically shaped quantum dots

    Energy Technology Data Exchange (ETDEWEB)

    Duque, C.M.; Morales, A.L. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia); Mora-Ramos, M.E. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia); Facultad de Ciencias, Universidad Autónoma del Estado de Morelos, Av. Universidad 1001, CP 62209 Cuernavaca, Morelos (Mexico); Duque, C.A. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia)

    2014-10-15

    An investigation of the effects of the dilute nitrogen contents in the exciton states of cylindrical In{sub x}Ga{sub 1−x}N{sub y}As{sub 1−y}/GaAs quantum dots is presented. The exciton states in the system are obtained within the effective mass theory and the band anti-crossing model. Exciton-related nonlinear optical absorption and refractive index change, as well as excitonic photoluminescence are studied with the help of the calculated exciton states. - Highlights: • Theoretical study of excitons in cylindrical In{sub x}Ga{sub 1−x}N{sub y}As{sub 1−y}/GaAs quantum dots. • Calculations of binding energy for different configurations of electron-hole pairs. • Nonlinear optical absorption and refractive index changes. • Dependence of photoluminescence energy transitions with several inputs.

  9. Semiconductor quantum optics with tailored photonic nanostructures

    Energy Technology Data Exchange (ETDEWEB)

    Laucht, Arne

    2011-06-15

    This thesis describes detailed investigations of the effects of photonic nanostructures on the light emission properties of self-assembled InGaAs quantum dots. Nanoscale optical cavities and waveguides are employed to enhance the interaction between light and matter, i.e. photons and excitons, up to the point where optical non-linearities appear at the quantum (single photon) level. Such non-linearities are an essential component for the realization of hardware for photon based quantum computing since they can be used for the creation and detection of non-classical states of light and may open the way to new genres of quantum optoelectronic devices such as optical modulators and optical transistors. For single semiconductor quantum dots in photonic crystal nanocavities we investigate the coupling between excitonic transitions and the highly localized mode of the optical cavity. We explore the non-resonant coupling mechanisms which allow excitons to couple to the cavity mode, even when they are not spectrally in resonance. This effect is not observed for atomic cavity quantum electrodynamics experiments and its origin is traced to phonon-assisted scattering for small detunings ({delta}E<{proportional_to}5 meV) and a multi-exciton-based, Auger-like process for larger detunings ({delta}E >{proportional_to}5 meV). For quantum dots in high-Q cavities we observe the coherent coupling between exciton and cavity mode in the strong coupling regime of light-matter interaction, probe the influence of pure dephasing on the coherent interaction at high excitation levels and high lattice temperatures, and examine the coupling of two spatially separated quantum dots via the exchange of real and virtual photons mediated by the cavity mode. Furthermore, we study the spontaneous emission properties of quantum dots in photonic crystal waveguide structures, estimate the fraction of all photons emitted into the propagating waveguide mode, and demonstrate the on-chip generation of

  10. Nonlinear fiber gyroscope for quantum metrology

    CERN Document Server

    Luis, Alfredo; Rivas, Ángel

    2016-01-01

    We examine the performance of a nonlinear fiber gyroscope for improved signal detection beating the quantum limits of its linear counterparts. The performance is examined when the nonlinear gyroscope is illuminated by practical field states, such as coherent and quadrature squeezed states. This is compared with the case of more ideal probes such as photon-number states.

  11. Nonlinear fiber gyroscope for quantum metrology

    Science.gov (United States)

    Luis, Alfredo; Morales, Irene; Rivas, Ángel

    2016-07-01

    We examine the performance of a nonlinear fiber gyroscope for improved signal detection beating the quantum limits of its linear counterparts. The performance is examined when the nonlinear gyroscope is illuminated by practical field states, such as coherent and quadrature squeezed states. This is compared with the case of more ideal probes such as photon-number states.

  12. Terahertz Quantum Plasmonics of Nanoslot Antennas in Nonlinear Regime.

    Science.gov (United States)

    Kim, Joon-Yeon; Kang, Bong Joo; Park, Joohyun; Bahk, Young-Mi; Kim, Won Tae; Rhie, Jiyeah; Jeon, Hyeongtag; Rotermund, Fabian; Kim, Dai-Sik

    2015-10-14

    Quantum tunneling in plasmonic nanostructures has presented an interesting aspect of incorporating quantum mechanics into classical optics. However, the study has been limited to the subnanometer gap regime. Here, we newly extend quantum plasmonics to gap widths well over 1 nm by taking advantage of the low-frequency terahertz regime. Enhanced electric fields of up to 5 V/nm induce tunneling of electrons in different arrays of ring-shaped nanoslot antennas of gap widths from 1.5 to 10 nm, which lead to a significant nonlinear transmission decrease. These observations are consistent with theoretical calculations considering terahertz-funneling-induced electron tunneling across the gap.

  13. Combined effects of intense laser field, electric and magnetic fields on the nonlinear optical properties of the step-like quantum well

    Energy Technology Data Exchange (ETDEWEB)

    Kasapoglu, E., E-mail: ekasap@cumhuriyet.edu.tr [Department of Physics, Cumhuriyet University, 58140 Sivas (Turkey); Duque, C.A. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia-UdeA, Calle 70 No. 52-21, Medellín (Colombia); Mora-Ramos, M.E. [Facultad de Ciencias, Universidad Autónoma del Estado de Morelos, Ave. Universidad 1001, CP 62209, Cuernavaca, Morelos (Mexico); Restrepo, R.L. [Department of Physics, Cumhuriyet University, 58140 Sivas (Turkey); Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia-UdeA, Calle 70 No. 52-21, Medellín (Colombia); Escuela de Ingeniería de Antioquia-EIA, Medellín (Colombia); Ungan, F.; Yesilgul, U.; Sari, H. [Department of Physics, Cumhuriyet University, 58140 Sivas (Turkey); Sökmen, I. [Department of Physics, Dokuz Eylül University, 35160 Buca, İzmir (Turkey)

    2015-03-15

    In the present work, the effects of the intense laser field on total optical absorption coefficient (the linear and third-order nonlinear) and total refractive index change for transition between two lower-lying electronic levels in the step-like GaAs/Ga{sub 1−x}Al{sub x}As quantum well under external electric and magnetic fields are investigated. The calculations were performed within the compact density-matrix formalism with the use of the effective mass and parabolic band approximations. The obtained results show that both total absorption coefficient and refractive index change are sensitive to the well dimensions and the effects of external fields. By changing the intensities of the electric, magnetic and non-resonant intense laser fields together with the well dimensions, we can obtain the blue or red shift, without the need for the growth of many different samples. - Highlights: • Augmentation of laser-field results in red shift in total AC spectra. • Magnetic field induces a blue-shift in the resonant peak. • Resonant peak position shifts to red with effect of electric field. • Resonant peak of total AC shifts to the higher photon energies with increasing well width.

  14. Assessing the quantum mechanical level of theory for prediction of linear and nonlinear optical properties of push-pull organic molecules.

    Science.gov (United States)

    Paschoal, Diego; Santos, Hélio F Dos

    2013-05-01

    In this paper, we assessed the quantum mechanical level of theory for prediction of linear and nonlinear optical (NLO) properties of push-pull organic molecules. The electric dipole moment (μ), mean polarizability ([Symbol: see text]α[Symbol: see text]) and total static first hyperpolarizability (βt) were calculated for a set of benzene, styrene, biphenyl and stilbene derivatives using HF, MP2 and DFT (31 different functionals) levels and over 71 distinct basis sets. In addition, we propose two new basis sets, NLO-V and aNLO-V, for NLO properties calculations. As the main outcomes it is shown that long-range corrected DFT functionals such as M062X, ωB97, cam-B3LYP, LC-BLYP and LC-ωPBE work satisfactorily for NLO properties when appropriate basis sets such as those proposed here (NLO-V or aNLO-V) are used. For most molecules with β ranging from 0 to 190 esu, the average absolute deviation was 13.2 esu for NLO-V basis sets, compared to 27.2 esu for the standard 6-31 G(2d) basis set. Therefore, we conclude that the new basis sets proposed here (NLO-V and aNLO-V), together with the cam-B3LYP functional, make an affordable calculation scheme to predict NLO properties of large organic molecules.

  15. Unsymmetrical squaraines for nonlinear optical materials

    Science.gov (United States)

    Marder, Seth R. (Inventor); Chen, Chin-Ti (Inventor); Cheng, Lap-Tak (Inventor)

    1996-01-01

    Compositions for use in non-linear optical devices. The compositions have first molecular electronic hyperpolarizability (.beta.) either positive or negative in sign and therefore display second order non-linear optical properties when incorporated into non-linear optical devices.

  16. Quantum optical properties in plasmonic systems

    Science.gov (United States)

    Ooi, C. H. Raymond

    2015-04-01

    Plasmonic metallic particle (MP) can affect the optical properties of a quantum system (QS) in a remarkable way. We develop a general quantum nonlinear formalism with exact vectorial description for the scattered photons by the QS. The formalism enables us to study the variations of the dielectric function and photon spectrum of the QS with the particle distance between QS and MP, exciting laser direction, polarization and phase in the presence of surface plasmon resonance (SPR) in the MP. The quantum formalism also serves as a powerful tool for studying the effects of these parameters on the nonclassical properties of the scattered photons. The plasmonic effect of nanoparticles has promising possibilities as it provides a new way for manipulating quantum optical properties of light in nanophotonic systems.

  17. Models of optical quantum computing

    Directory of Open Access Journals (Sweden)

    Krovi Hari

    2017-03-01

    Full Text Available I review some work on models of quantum computing, optical implementations of these models, as well as the associated computational power. In particular, we discuss the circuit model and cluster state implementations using quantum optics with various encodings such as dual rail encoding, Gottesman-Kitaev-Preskill encoding, and coherent state encoding. Then we discuss intermediate models of optical computing such as boson sampling and its variants. Finally, we review some recent work in optical implementations of adiabatic quantum computing and analog optical computing. We also provide a brief description of the relevant aspects from complexity theory needed to understand the results surveyed.

  18. Non-linear (loop) quantum cosmology

    CERN Document Server

    Bojowald, Martin; Dantas, Christine C; Jaffe, Matthew; Simpson, David

    2012-01-01

    Inhomogeneous quantum cosmology is modeled as a dynamical system of discrete patches, whose interacting many-body equations can be mapped to a non-linear minisuperspace equation by methods analogous to Bose-Einstein condensation. Complicated gravitational dynamics can therefore be described by more-manageable equations for finitely many degrees of freedom, for which powerful solution procedures are available, including effective equations. The specific form of non-linear and non-local equations suggests new questions for mathematical and computational investigations, and general properties of non-linear wave equations lead to several new options for physical effects and tests of the consistency of loop quantum gravity. In particular, our quantum cosmological methods show how sizeable quantum corrections in a low-curvature universe can arise from tiny local contributions adding up coherently in large regions.

  19. Quantum optics. Gravity meets quantum physics

    Energy Technology Data Exchange (ETDEWEB)

    Adams, Bernhard W. [Argonne National Lab. (ANL), Argonne, IL (United States)

    2015-02-27

    Albert Einstein’s general theory of relativity is a classical formulation but a quantum mechanical description of gravitational forces is needed, not only to investigate the coupling of classical and quantum systems but simply to give a more complete description of our physical surroundings. In this issue of Nature Photonics, Wen-Te Liao and Sven Ahrens reveal a link between quantum and gravitational physics. They propose that in the quantum-optical effect of superradiance, the world line of electromagnetic radiation is changed by the presence of a gravitational field.

  20. Second-order nonlinear optical susceptibilities induced by built-in electric field in wurtzite nitride double quantum wells

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, L. [State Key Laboratory for Mesoscopic Physics, and School of Physics, Peking University, Beijing 100871 (China) and Department of Mechanism and Electron, Panyu Polytechnic, Panyu 511483 (China)]. E-mail: zhangli-gz@263.net; Chi Yuemeng [State Key Laboratory for Mesoscopic Physics, and School of Physics, Peking University, Beijing 100871 (China); Shi, J.-J. [State Key Laboratory for Mesoscopic Physics, and School of Physics, Peking University, Beijing 100871 (China)

    2007-06-25

    Based on the density matrix method and the iterative treatment, the second-harmonic generation (SHG) susceptibility of a wurtzite nitride coupling quantum well (CQW) with strong built-in electric fields have been theoretically investigated. The effect of the band non-parabolicity effect has been taken into account. A typical wurtzite GaN/In{sub x}Ga{sub 1-x}N CQW are chosen to perform numerical calculations. The localized properties of the electronic ground state and the low-excited states in the system are analyzed in detail. The calculated SHG coefficients reach the order of magnitude of 10{sup -7}m/V, which is two-order larger than the corresponding values in wurtzite single quantum wells. Moreover, it is confirmed that the SHG coefficients are not monotonic functions of the well width, barrier width and the doped concentration of the CQW systems, but have complicated dependent relations on them. The reasons resulting in these characteristics can be attributed to the intense competition between the strong built-in electric field effect and the quantum size effect for the electronic confined situation in the wurtzite CQWs. The calculated results also show that a strong SHG effect can be realized in the nitride CQW by choosing a group of optimized structural parameters and doped fraction.

  1. Single-cycle nonlinear optics

    Energy Technology Data Exchange (ETDEWEB)

    Max-Planck-Institut fur Quantenoptik; Goulielmakis, E.; Schultze, M.; Hofstetter, M.; Yakovlev, V. S.; Gagnon, J.; Uiberacker, M.; Aquila, A. L.; gullikson, E. M.; attwood, D. T.; Kienberger, R.; Krausz, F.; Kleineberg, U.

    2008-11-05

    Nonlinear optics plays a central role in the advancement of optical science and laser-based technologies. We report on the confinement of the nonlinear interaction of light with matter to a single wave cycle and demonstrate its utility for time-resolved and strong-field science. The electric field of 3.3-femtosecond, 0.72-micron laser pulses with a controlled and measured waveform ionizes atoms near the crests of the central wave cycle, with ionization being virtually switched off outside this interval. Isolated sub-100-attosecond pulses of extreme ultraviolet light (photon energy {approx} 80 electron volts), containing {approx} 0.5 nanojoule of energy, emerge from the interaction with a conversion efficiency of {approx} 10{sup -6}. These tools enable the study of the precision control of electron motion with light fields and electron-electron interactions with a resolution approaching the atomic unit of time ({approx} 24 attoseconds).

  2. Introduction to modern quantum optics

    CERN Document Server

    Peng Jin Sheng

    1998-01-01

    This book discusses quantum optics and investigates the quantum properties of interactions between atoms and laser fields. It is divided into three parts. Part I introduces the elementary theory of the interaction between atoms and light. Part II provides a concentrated discussion on the quantum properties of light fields. Part III deals with the quantum dynamic properties of the atoms interacting with laser fields. This book can be used as a text for both graduate and undergraduate students; it will also benefit scientists who are interested in quantum optics and theoretical physics.

  3. Linear optics and quantum maps

    CERN Document Server

    Aiello, A; Woerdman, J P

    2006-01-01

    We present a theoretical analysis of the connection between classical polarization optics and quantum mechanics of two-level systems. First, we review the matrix formalism of classical polarization optics from a quantum information perspective. In this manner the passage from the Stokes-Jones-Mueller description of classical optical processes to the representation of one- and two-qubit quantum operations, becomes straightforward. Second, as a practical application of our classical-\\emph{vs}-quantum formalism, we show how two-qubit maximally entangled mixed states (MEMS), can be generated by using polarization and spatial modes of photons generated via spontaneous parametric down conversion.

  4. Quantum cryptography using optical fibers.

    Science.gov (United States)

    Franson, J D; Lives, H

    1994-05-10

    Quantum cryptography permits the transmission of secret information whose security is guaranteed by the uncertainty principle. An experimental system for quantum crytography is implemented based on the linear polarization of single photons transmitted by an optical fiber. Polarization-preserving optical fiber and a feedback loop are employed to maintain the state of polarization. Error rates of less than 0.5% are obtained.

  5. Organosilicon Polymeric Nonlinear Optical Materials for Optical Switching and Modulation

    Science.gov (United States)

    1994-02-28

    Organosilicon Polymeric Nonlinear Optical Materials for Optical C: F49620-93-C-0039 Switching and Modulation 6. AUTHOR(S) Mr. Sandip K. Sengupta, Dr...D FINAL REPORT for Organosilicon Polymeric Nonlinear Optical Materials for Optical Switching and Modulation Prepared for: USAF, AFMC (AFOSR) Air Force...34Organosilicon Polymeric Nonlinear Optical Materials for Optical Switching and Modulation," contract number F49620-93-C-0039. The work has been performed by Dr

  6. Extra phase noise from thermal fluctuations in nonlinear optical crystals

    DEFF Research Database (Denmark)

    César, J. E. S.; Coelho, A.S.; Cassemiro, K.N.

    2009-01-01

    We show theoretically and experimentally that scattered light by thermal phonons inside a second-order nonlinear crystal is the source of additional phase noise observed in optical parametric oscillators. This additional phase noise reduces the quantum correlations and has hitherto hindered the d...... the direct production of multipartite entanglement in a single nonlinear optical system. We cooled the nonlinear crystal and observed a reduction in the extra noise. Our treatment of this noise can be successfully applied to different systems in the literature....

  7. Nonlinear optical interactions in silicon waveguides

    Science.gov (United States)

    Kuyken, B.; Leo, F.; Clemmen, S.; Dave, U.; Van Laer, R.; Ideguchi, T.; Zhao, H.; Liu, X.; Safioui, J.; Coen, S.; Gorza, S. P.; Selvaraja, S. K.; Massar, S.; Osgood, R. M.; Verheyen, P.; Van Campenhout, J.; Baets, R.; Green, W. M. J.; Roelkens, G.

    2017-03-01

    The strong nonlinear response of silicon photonic nanowire waveguides allows for the integration of nonlinear optical functions on a chip. However, the detrimental nonlinear optical absorption in silicon at telecom wavelengths limits the efficiency of many such experiments. In this review, several approaches are proposed and demonstrated to overcome this fundamental issue. By using the proposed methods, we demonstrate amongst others supercontinuum generation, frequency comb generation, a parametric optical amplifier, and a parametric optical oscillator.

  8. Graphene - a rather ordinary nonlinear optical material

    CERN Document Server

    khurgin, Jacob B

    2014-01-01

    An analytical expression for the nonlinear refractive index of graphene has been derived and used to obtain the performance metrics of third order nonlinear devices using graphene as a nonlinear medium. None of the metrics is found to be superior to the existing nonlinear optical materials.

  9. Donor impurity-related linear and nonlinear optical absorption coefficients in GaAs/Ga{sub 1−x}Al{sub x}As concentric double quantum rings: Effects of geometry, hydrostatic pressure, and aluminum concentration

    Energy Technology Data Exchange (ETDEWEB)

    Baghramyan, H.M.; Barseghyan, M.G.; Kirakosyan, A.A. [Department of Solid State Physics, Yerevan State University, Al. Manookian 1, 0025 Yerevan (Armenia); Restrepo, R.L. [Física Teórica y Aplicada, Escuela de Ingeniería de Antioquia, AA 7516, Medellín (Colombia); Grupo de Materia Condensada-UdeA, Instituto de Física, Facultadde Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21,Medellín (Colombia); Mora-Ramos, M.E. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultadde Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21,Medellín (Colombia); Facultad de Ciencias, Universidad Autónoma del Estado de Morelos, Av. Universidad 1001, CP 62209, Cuernavaca, Morelos (Mexico); Duque, C.A., E-mail: cduque@fisica.udea.edu.co [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultadde Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21,Medellín (Colombia)

    2014-01-15

    The linear and nonlinear optical absorption associated with the transition between 1s and 2s states corresponding to the electron-donor-impurity complex in GaAs/Ga{sub 1−x}Al{sub x}As three-dimensional concentric double quantum rings are investigated. Taking into account the combined effects of hydrostatic pressure and the variation of the aluminum concentration, the energies of the ground and first excited s-like states of a donor impurity in such a system have been calculated using the effective mass approximation and a variational method. The energies of these states and the corresponding threshold energy of the optical transitions are examined as functions of hydrostatic pressure, aluminum concentration, radial impurity position, as well as the geometrical dimensions of the structure. The dependencies of the linear, nonlinear and total optical absorption coefficients as functions of the incident photon energy are investigated for different values of those mentioned parameters. It is found that the influences mentioned above lead to either redshifts or blueshifts of the resonant peaks of the optical absorption spectrum. It is particularly discussed the unusual property exhibited by the third-order nonlinear of becoming positive for photon energies below the resonant transition one. It is shown that this phenomenon is associated with the particular features of the system under study, which determine the values of the electric dipole moment matrix elements. -- Highlights: • Intra-band optical absorption associated to impurity states in double quantum rings. • Combined effects of hydrostatic pressure and aluminum concentration are studied. • The influences mentioned above lead to shifts of resonant peaks. • It is discussed an unusual property exhibited by the third-order nonlinear absorption.

  10. Nonlinear optical crystals a complete survey

    CERN Document Server

    Nikogosyan, David N

    2005-01-01

    Nonlinear optical crystals are widely used in modern optical science and technology for frequency conversion of laser light, i.e. to generate laser radiation at any specific wavelength in visible, UV or IR spectral regions. This unrivalled reference book contains the most complete and up-to-date information on properties of nonlinear optical crystals. It includes: * Database of 63 common and novel nonlinear optical crystals * Periodically-poled and self-frequency-doubling materials * Full description of linear and nonlinear optical properties * Significant amount of crystallophysical, thermophysical, spectroscopic, electro-optic and magneto-optic information * 7 mini-reviews on novel applications, such as deep-UV light generation, terahertz-wave generation, ultrashort laser pulse compression, photonic band-gap crystals, x3 nonlinearity, etc. * More than 1500 different references with full titles It is a vital source of information for scientists and engineers dealing with modern applications of nonlinear opti...

  11. Performance Analysis of High-speed Optical Pulse Transmission in Dispersion-managed Nonlinear Birefringent Fiber Using Quantum Well Laser Diode Sources

    Institute of Scientific and Technical Information of China (English)

    YAN Minhui; CHEN Jianping

    2002-01-01

    This paper analyzes the high bit-rate optical pulse trasmission in single mode optical fiber with chromatic dispersion, polarization mode dispersion (small random birefringence) and nonlinearity. Numerical method employed can precisely describe their interactive effect on transmission performance. Different dispersion maps and the related performance are analysed. Various simulation results and discussion are given. The results show that chromatic dispersion compensation should be carefully designed. Appropriate dispersion management can also alleviate the effect of polarization mode dispersion.

  12. Contactless nonlinear optics mediated by long-range Rydberg interactions

    Science.gov (United States)

    Busche, Hannes; Huillery, Paul; Ball, Simon W.; Ilieva, Teodora; Jones, Matthew P. A.; Adams, Charles S.

    2017-07-01

    In conventional nonlinear optics, linear quantum optics, and cavity quantum electrodynamics to create effective photon-photon interactions photons must have, at one time, interacted with matter inside a common medium. In contrast, in Rydberg quantum optics, optical photons are coherently and reversibly mapped onto collective atomic Rydberg excitations, giving rise to dipole-mediated effective photon-photon interactions that are long range. Consequently, a spatial overlap between the light modes is no longer required. We demonstrate such a contactless coupling between photons stored as collective Rydberg excitations in spatially separate optical media. The potential induced by each photon modifies the retrieval mode of its neighbour, leading to correlations between them. We measure these correlations as a function of interaction strength, distance and storage time, demonstrating an effective interaction between photons separated by 15 times their wavelength. Contactless effective photon-photon interactions are relevant for scalable multichannel photonic devices and the study of strongly correlated many-body dynamics using light.

  13. Optically active quantum dots

    Science.gov (United States)

    Gerard, Valerie; Govan, Joseph; Loudon, Alexander; Baranov, Alexander V.; Fedorov, Anatoly V.; Gun'ko, Yurii K.

    2015-10-01

    The main goal of our research is to develop new types of technologically important optically active quantum dot (QD) based materials, study their properties and explore their biological applications. For the first time chiral II-VI QDs have been prepared by us using microwave induced heating with the racemic (Rac), D- and L-enantiomeric forms of penicillamine as stabilisers. Circular dichroism (CD) studies of these QDs have shown that D- and L-penicillamine stabilised particles produced mirror image CD spectra, while the particles prepared with a Rac mixture showed only a weak signal. It was also demonstrated that these QDs show very broad emission bands between 400 and 700 nm due to defects or trap states on the surfaces of the nanocrystals. These QDs have demonstrated highly specific chiral recognition of various biological species including aminoacids. The utilisation of chiral stabilisers also allowed the preparation of new water soluble white emitting CdS nano-tetrapods, which demonstrated circular dichroism in the band-edge region of the spectrum. Biological testing of chiral CdS nanotetrapods displayed a chiral bias for an uptake of the D- penicillamine stabilised nano-tetrapods by cancer cells. It is expected that this research will open new horizons in the chemistry of chiral nanomaterials and their application in nanobiotechnology, medicine and optical chemo- and bio-sensing.

  14. Euclidean Quantum Mechanics and Universal Nonlinear Filtering

    Directory of Open Access Journals (Sweden)

    Bhashyam Balaji

    2009-02-01

    Full Text Available An important problem in applied science is the continuous nonlinear filtering problem, i.e., the estimation of a Langevin state that is observed indirectly. In this paper, it is shown that Euclidean quantum mechanics is closely related to the continuous nonlinear filtering problem. The key is the configuration space Feynman path integral representation of the fundamental solution of a Fokker-Planck type of equation termed the Yau Equation of continuous-continuous filtering. A corollary is the equivalence between nonlinear filtering problem and a time-varying Schr¨odinger equation.

  15. Nonlinear peltier effect in quantum point contacts

    Science.gov (United States)

    Bogachek, E. N.; Scherbakov, A. G.; Landman, Uzi

    1998-11-01

    A theoretical analysis of the Peltier effect in two-dimensional quantum point contacts, in field-free conditions and under the influence of applied magnetic fields, is presented. It is shown that in the nonlinear regime (finite applied voltage) new peaks in the Peltier coefficient appear leading to violation of Onsager's relation. Oscillations of the Peltier coefficient in a magnetic field are demonstrated.

  16. Thermal rectification in nonlinear quantum circuits

    DEFF Research Database (Denmark)

    Ruokola, T.; Ojanen, T.; Jauho, Antti-Pekka

    2009-01-01

    We present a theoretical study of radiative heat transport in nonlinear solid-state quantum circuits. We give a detailed account of heat rectification effects, i.e., the asymmetry of heat current with respect to a reversal of the thermal gradient, in a system consisting of two reservoirs at finite...

  17. Quantum Optics Including Noise Reduction, Trapped Ions, Quantum Trajectories, and Decoherence

    CERN Document Server

    Orszag, Miguel

    2008-01-01

    Quantum Optics gives a very broad coverage of basic laser-related phenomena that allow scientist and engineers to carry out research in quantum optics and laser physics. It covers quantization of the electromagnetic field, quantum theory of coherence, atom-field interaction models, resonance fluorescence, quantum theory of damping, laser theory using both the master equation and the Langevin theory, the correlated emission laser, input-output theory with applications to non-linear optics, quantum trajectories, quantum non-demolition measurements and generation of non-classical vibrational states of ions in a Paul trap. In this second edition, there is an enlarged chapter on decoherence, as well as additional material dealing with elements of quantum computation, entanglement of pure and mixed states as well as a chapter on quantum copying and processors. These topics are presented in a unified and didactic manner. The presentation of the book is clear and pedagogical; it balances the theoretical aspect of qua...

  18. Linear optics implementation for quantum game under quantum noise

    Institute of Scientific and Technical Information of China (English)

    Cao Shuai; Fang Mao-Fa

    2006-01-01

    It has recently been shown that linear optics alone would suffice to implement efficient quantum computation. Quantum computation circuits using coherent states as the logical qubits can be constructed from very simple linear networks, conditional measurements and coherent superposition resource states. We present the quantum game under quantum noise and a proposal for implementing the noisy quantum game using only linear optics.

  19. Harmonic nanoparticles: noncentrosymmetric metal oxides for nonlinear optics

    OpenAIRE

    Rogov, Andrii; Mugnier, Yannick; Bonacina, Luigi

    2015-01-01

    The combination of nonlinear optics and nanotechnology is an extremely rich scientific domain yet widely unexplored. We present here a review of recent optical investigations on noncentrosymmetric oxide nanoparticles with a large ${{\\chi }^{(2)}}$ response, often referred to as harmonic nanoparticles (HNPs). HNPs feature a series of properties which distinguish them from other photonics nanoprobes (quantum dots, up-conversion nanoparticles, noble metal particles). HNPs emission is inherently ...

  20. Nonlinear Photonics and Novel Optical Phenomena

    CERN Document Server

    Morandotti, Roberto

    2012-01-01

    Nonlinear Photonics and Novel Optical Phenomena contains contributed chapters from leading experts in nonlinear optics and photonics, and provides a comprehensive survey of fundamental concepts as well as hot topics in current research on nonlinear optical waves and related novel phenomena. The book covers self-accelerating airy beams, integrated photonics based on high index doped-silica glass, linear and nonlinear spatial beam dynamics in photonic lattices and waveguide arrays, polariton solitons and localized structures in semiconductor microcavities, terahertz waves, and other novel phenomena in different nanophotonic and optical systems.

  1. Fibre-optic nonlinear optical microscopy and endoscopy.

    Science.gov (United States)

    Fu, L; Gu, M

    2007-06-01

    Nonlinear optical microscopy has been an indispensable laboratory tool of high-resolution imaging in thick tissue and live animals. Rapid developments of fibre-optic components in terms of growing functionality and decreasing size provide enormous opportunities for innovations in nonlinear optical microscopy. Fibre-based nonlinear optical endoscopy is the sole instrumentation to permit the cellular imaging within hollow tissue tracts or solid organs that are inaccessible to a conventional optical microscope. This article reviews the current development of fibre-optic nonlinear optical microscopy and endoscopy, which includes crucial technologies for miniaturized nonlinear optical microscopy and their embodiments of endoscopic systems. A particular attention is given to several classes of photonic crystal fibres that have been applied to nonlinear optical microscopy due to their unique properties for ultrashort pulse delivery and signal collection. Furthermore, fibre-optic nonlinear optical imaging systems can be classified into portable microscopes suitable for imaging behaving animals, rigid endoscopes that allow for deep tissue imaging with minimally invasive manners, and flexible endoscopes enabling imaging of internal organs. Fibre-optic nonlinear optical endoscopy is coming of age and a paradigm shift leading to optical microscope tools for early cancer detection and minimally invasive surgery.

  2. The effects of the intense laser field on the nonlinear optical properties of a cylindrical Ga{sub 1−x}Al{sub x}As/GaAs quantum dot under applied electric field

    Energy Technology Data Exchange (ETDEWEB)

    Kasapoglu, E., E-mail: ekasap@cumhuriyet.edu.tr [Department of Physics, Cumhuriyet University, 58140 Sivas (Turkey); Duque, C.A. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia); Mora-Ramos, M.E. [Centro de Investigación en Ciencias, Instituto de Ciencias Básicas y Aplicadas, Universidad Autóonoma del Estado de Morelos, Av. Universidad 1001, CP 62209 Cuernavaca, Morelos (Mexico); Sökmen, I. [Department of Physics, Dokuz Eylül University, 35160 Buca, İzmir (Turkey)

    2015-10-01

    In the present work, the effects of the intense laser field on total optical absorption coefficient (the linear and third-order nonlinear) and total refractive index change (the linear and third-order nonlinear) for transitions between different intersubbands in the Ga{sub 1−x}Al{sub x}As/GaAs cylindrical quantum dot under external electric field are investigated. The calculations were performed within the compact density-matrix formalism with the use of the effective mass approximation. The obtained results show that both total absorption coefficient and refractive index change are sensitive to the electric and intense laser fields. By changing the intensities of the electric and laser fields, we can obtain the blue or red shift, without the need for the growth of many different samples. - Highlights: • The effects of the non-resonant intense laser field and electric field on the nonlinear optical properties of cylindrical quantum dot are investigated. • The both total absorption coefficient and refractive index change are sensitive to dot dimensions and the effects of external fields. • By changing the external fields together with dot dimensions a blue or red shift can be obtained.

  3. Interaction-based nonlinear quantum metrology with a cold atomic ensemble

    OpenAIRE

    2014-01-01

    In this manuscript we present an experimental and theoretical investigation of quantum-noise-limited measurement by nonlinear interferometry, or from another perspective, quantum-noise-limited interaction-based measurement. The experimental work is performed using a polarization-based quantum interface between propagating light pulses and cold rubidium-87 atoms trapped in an optical dipole trap. We first review the theory of quantum metrology and estimation theory, and we describe theor...

  4. Electrifying photonic metamaterials for tunable nonlinear optics.

    Science.gov (United States)

    Kang, Lei; Cui, Yonghao; Lan, Shoufeng; Rodrigues, Sean P; Brongersma, Mark L; Cai, Wenshan

    2014-08-11

    Metamaterials have not only enabled unprecedented flexibility in producing unconventional optical properties that are not found in nature, they have also provided exciting potential to create customized nonlinear media with high-order properties correlated to linear behaviour. Two particularly compelling directions are active metamaterials, whose optical properties can be purposely tailored by external stimuli in a reversible manner, and nonlinear metamaterials, which enable intensity-dependent frequency conversion of light waves. Here, by exploring the interaction of these two directions, we leverage the electrical and optical functions simultaneously supported in nanostructured metals and demonstrate electrically controlled nonlinear optical processes from a metamaterial. Both second harmonic generation and optical rectification, enhanced by the resonance behaviour in the metamaterial absorber, are modulated externally with applied voltage signals. Our results reveal an opportunity to exploit optical metamaterials as self-contained, dynamic electro-optic systems with intrinsically embedded electrical functions and optical nonlinearities.

  5. Quantum information processing in nanostructures Quantum optics; Quantum computing

    CERN Document Server

    Reina-Estupinan, J H

    2002-01-01

    Since information has been regarded os a physical entity, the field of quantum information theory has blossomed. This brings novel applications, such as quantum computation. This field has attracted the attention of numerous researchers with backgrounds ranging from computer science, mathematics and engineering, to the physical sciences. Thus, we now have an interdisciplinary field where great efforts are being made in order to build devices that should allow for the processing of information at a quantum level, and also in the understanding of the complex structure of some physical processes at a more basic level. This thesis is devoted to the theoretical study of structures at the nanometer-scale, 'nanostructures', through physical processes that mainly involve the solid-state and quantum optics, in order to propose reliable schemes for the processing of quantum information. Initially, the main results of quantum information theory and quantum computation are briefly reviewed. Next, the state-of-the-art of ...

  6. Few-photon coherent nonlinear optics with a single molecule

    CERN Document Server

    Maser, Andreas; Utikal, Tobias; Götzinger, Stephan; Sandoghdar, Vahid

    2015-01-01

    The pioneering experiments of linear spectroscopy were performed using flames in the 1800s, but nonlinear optical measurements had to wait until lasers became available in the twentieth century. Because the nonlinear cross section of materials is very small, usually macroscopic bulk samples and pulsed lasers are used. Numerous efforts have explored coherent nonlinear signal generation from individual nanoparticles or small atomic ensembles with millions of atoms. Experiments on a single semiconductor quantum dot have also been reported, albeit with a very small yield. Here, we report on coherent nonlinear spectroscopy of a single molecule under continuous-wave single-pass illumination, where efficient photon-molecule coupling in a tight focus allows switching of a laser beam by less than a handful of pump photons nearly resonant with the sharp molecular transition. Aside from their fundamental importance, our results emphasize the potential of organic molecules for applications such as quantum information pro...

  7. Optical Implementation of Quantum Orienteering

    Science.gov (United States)

    Jeffrey, Evan R.; Altepeter, Joseph B.; Colci, Madalina; Kwiat, Paul G.

    2006-04-01

    We present results from an optical implementation of quantum orienteering, a protocol for communicating directions in space using quantum bits. We show how different types of measurements and encodings can be used to increase the communication efficiency. In particular, if Alice and Bob use two spin-1/2 particles for communication and employ joint measurements, they do better than is possible with local operations and classical communication. Furthermore, by using oppositely oriented spins, the achievable communication efficiency is further increased. Finally, we discuss the limitations of an optical approach: our results highlight the usually overlooked nonequivalence of different physical encodings of quantum bits.

  8. Optical Coherence and Quantum Optics

    CERN Document Server

    Mandel, Leonard

    1995-01-01

    This book presents a systematic account of optical coherence theory within the framework of classical optics, as applied to such topics as radiation from sources of different states of coherence, foundations of radiometry, effects of source coherence on the spectra of radiated fields, coherence theory of laser modes, and scattering of partially coherent light by random media. The book starts with a full mathematical introduction to the subject area and each chapter concludes with a set of exercises. The authors are renowned scientists and have made substantial contributions to many of the topi

  9. Hydrogenic impurity, external electric and magnetic fields effects on the nonlinear optical properties of a multi-layer spherical quantum dot

    Science.gov (United States)

    Tanhaei, M. H.; Rezaei, G.

    2016-10-01

    In this work, effects of an on-center hydrogenic impurity, external electric and magnetic fields on the optical rectification coefficient (ORC), second and third harmonic generations (SHG and THG) of a multi-layer spherical quantum dot (MLSQD) are studied. Energy eigenvalues and eigenvectors are calculated using the direct matrix diagonalization method and optical properties are obtained using the compact density matrix approach. Our results reveal that the hydrogenic impurity and external fields have a great influence on these optical quantities. Hydrogenic impurity reduces the magnitude of the resonant peaks and shifts them to the higher energies. An increase in the magnetic (electric) field, leads to increase (decrease) the interval energies and the dipole moment matrix elements. Therefore, resonant peaks of these optical quantities find an obvious blue (red) shift and their magnitudes enhance (diminish) with increasing the external magnetic (electric) field.

  10. Advances in nonlinear optical materials and devices

    Science.gov (United States)

    Byer, Robert L.

    1991-01-01

    The recent progress in the application of nonlinear techniques to extend the frequency of laser sources has come from the joint progress in laser sources and in nonlinear materials. A brief summary of the progress in diode pumped solid state lasers is followed by an overview of progress in nonlinear frequency extension by harmonic generation and parametric processes. Improved nonlinear materials including bulk crystals, quasiphasematched interactions, guided wave devices, and quantum well intersubband studies are discussed with the idea of identifying areas of future progress in nonlinear materials and devices.

  11. Design of Organic Nonlinear Optical Materials

    Science.gov (United States)

    1990-06-01

    This project deals with a new approach to designing organic nonlinear optical materials for second harmonic generation based on the use of hydrogen...patterns for even simple organic molecules. For organic nonlinear optical materials this dilemma means that even the most promising organic molecule may

  12. Quantum optics including noise reduction, trapped ions, quantum trajectories, and decoherence

    CERN Document Server

    Orszag, Miguel

    2016-01-01

    This new edition gives a unique and broad coverage of basic laser-related phenomena that allow graduate students, scientists and engineers to carry out research in quantum optics and laser physics. It covers quantization of the electromagnetic field, quantum theory of coherence, atom-field interaction models, resonance fluorescence, quantum theory of damping, laser theory using both the master equation and the Langevin theory, the correlated emission laser, input-output theory with applications to non-linear optics, quantum trajectories, quantum non-demolition measurements and generation of non-classical vibrational states of ions in a Paul trap. In this third edition, there is an enlarged chapter on trapped ions, as well as new sections on quantum computing and quantum bits with applications. There is also additional material included for quantum processing and entanglement. These topics are presented in a unified and didactic manner, each chapter is accompanied by specific problems and hints to solutions to...

  13. Non-linear excitation of quantum emitters in two-dimensional hexagonal boron nitride

    CERN Document Server

    Schell, Andreas W; Takashima, Hideaki; Takeuchi, Shigeki; Aharonovich, Igor

    2016-01-01

    Two-photon absorption is an important non-linear process employed for high resolution bio-imaging and non-linear optics. In this work we realize two-photon excitation of a quantum emitter embedded in a two-dimensional material. We examine defects in hexagonal boron nitride and show that the emitters exhibit similar spectral and quantum properties under one-photon and two-photon excitation. Furthermore, our findings are important to deploy two-dimensional hexagonal boron nitride for quantum non-linear photonic applications.

  14. Quantum optics with quantum dots in photonic nanowires

    DEFF Research Database (Denmark)

    We will review recent studies performed on InAs quantum dots embedded in GaAs photonic wires, which highlight the strong interest of the photonic wire geometry for quantum optics experiments and quantum optoelectronic devices.......We will review recent studies performed on InAs quantum dots embedded in GaAs photonic wires, which highlight the strong interest of the photonic wire geometry for quantum optics experiments and quantum optoelectronic devices....

  15. Quantum Optics with Quantum Dots in Photonic Nanowires

    DEFF Research Database (Denmark)

    Gérard, J.-M.; Claudon, J.; Bleuse, J.;

    2011-01-01

    We review recent studies performed on InAs quantum dots embedded in GaAs photonic wires, which highlight the strong interest of the photonic wire geometry for quantum optics experiments and quantum optoelectronic devices.......We review recent studies performed on InAs quantum dots embedded in GaAs photonic wires, which highlight the strong interest of the photonic wire geometry for quantum optics experiments and quantum optoelectronic devices....

  16. Nonlinear dynamics and quantum chaos an introduction

    CERN Document Server

    Wimberger, Sandro

    2014-01-01

    The field of nonlinear dynamics and chaos has grown very much over the last few decades and is becoming more and more relevant in different disciplines. This book presents a clear and concise introduction to the field of nonlinear dynamics and chaos, suitable for graduate students in mathematics, physics, chemistry, engineering, and in natural sciences in general. It provides a thorough and modern introduction to the concepts of Hamiltonian dynamical systems' theory combining in a comprehensive way classical and quantum mechanical description. It covers a wide range of topics usually not found in similar books. Motivations of the respective subjects and a clear presentation eases the understanding. The book is based on lectures on classical and quantum chaos held by the author at Heidelberg University. It contains exercises and worked examples, which makes it ideal for an introductory course for students as well as for researchers starting to work in the field.

  17. Quantum Optics with Quantum Dots in Photonic Nanowires

    DEFF Research Database (Denmark)

    Gérard, J. M.; Claudon, J.; Bleuse, J.;

    2012-01-01

    We review recent experimental and theoretical results, which highlight the strong interest of the photonic wire geometry for solid-state quantum optics and quantum optoelectronic devices.......We review recent experimental and theoretical results, which highlight the strong interest of the photonic wire geometry for solid-state quantum optics and quantum optoelectronic devices....

  18. Photoconductive and nonlinear optical properties of composites based on metallophthalocyanines

    Science.gov (United States)

    Vannikov, A. V.; Grishina, A. D.; Gorbunova, Yu. G.; Tsivadze, A. Yu.

    2015-08-01

    The photoconductive, photorefractive and nonlinear optical properties of composites from polyvinylcarbazole or aromatic polyimide containing supramolecular ensembles of (tetra-15-crown-5) - phthalocyaninato gallium, indium, - phthalocyaninateacetato yttrium, - phthalocyaninato ruthenium with axially coordinated pyrazine molecules were investigated at 633, 1030 and 1064nmusing continuous and pulsed lasers. Supramolecular ensembles (SE) were prepared through dissolution of molecular metallophthalocyanines in tetrachloroethane (TCE) and subsequent treatment via three cycles of heating to 90∘C and slow cooling to room temperature. The zscan method in femtosecond and nanosecond regimeswas used for measuring nonlinear optical properties phthalocyaninato indium and yttrium in TCE solutions and polymer films. It was established that effect of heavy metallic atom is basic factor which determines the quantum yield, photorefractive amplification of laser object beam, dielectric susceptibility of third order and nonlinear optical properties of metallophthalocyanines.

  19. Ultra-Low Power Optical Transistor Using a Single Quantum Dot Embedded in a Photonic Wire

    DEFF Research Database (Denmark)

    Nguyen, H.A.; Grange, T.; Malik, N.S.

    2017-01-01

    Using a single InAs quantum dot embedded in a GaAs photonic wire, we realize a giant non-linearity between two optical modes to experimentally demonstrate an all-optical transistor triggered by 10 photons.......Using a single InAs quantum dot embedded in a GaAs photonic wire, we realize a giant non-linearity between two optical modes to experimentally demonstrate an all-optical transistor triggered by 10 photons....

  20. Modulatable optical radiators and metasurfaces based on quantum nanoantennas

    KAUST Repository

    Chen, Pai-Yen

    2015-01-20

    We investigate the tunable and switchable optical radiators and metamaterials formed by metallic nanodipole antennas with submicroscopic gaps (1.2 nm), of which linear and third-order nonlinear quantum conductivities are observed due to the photon-assisted tunneling effect. The quantum conductivities induced at the nanogap are relevant to power dissipations, which can be enhanced by the strongly localized optical fields associated with the plasmonic resonance. We demonstrate that the scattering property of an individual quantum nanoantenna and the transparency of a metamasurface constituted of it can be tuned by electrostatically controlling the linear conductivity (electronic tuning) or by adjusting the irradiation intensity that varies the nonlinear quantum conductivity (all-optical tuning).

  1. A nonlinear Schroedinger wave equation with linear quantum behavior

    Energy Technology Data Exchange (ETDEWEB)

    Richardson, Chris D.; Schlagheck, Peter; Martin, John; Vandewalle, Nicolas; Bastin, Thierry [Departement de Physique, University of Liege, 4000 Liege (Belgium)

    2014-07-01

    We show that a nonlinear Schroedinger wave equation can reproduce all the features of linear quantum mechanics. This nonlinear wave equation is obtained by exploring, in a uniform language, the transition from fully classical theory governed by a nonlinear classical wave equation to quantum theory. The classical wave equation includes a nonlinear classicality enforcing potential which when eliminated transforms the wave equation into the linear Schroedinger equation. We show that it is not necessary to completely cancel this nonlinearity to recover the linear behavior of quantum mechanics. Scaling the classicality enforcing potential is sufficient to have quantum-like features appear and is equivalent to scaling Planck's constant.

  2. Nonlinear optical properties of ultrathin metal layers

    DEFF Research Database (Denmark)

    Lysenko, Oleg

    2016-01-01

    . The optical characterization of the plasmonic waveguides is performed using femtosecond and picosecond optical pulses. Two nonlinear optical effects in the strip plasmonic waveguides are experimentally observed and reported. The first effect is the nonlinear power transmission of the plasmonic mode......-order nonlinear susceptibility of the plasmonic mode in the gold strip waveguides significantly depends on the metal layer thickness and laser pulse duration. This dependence is explained in detail in terms of the free-electron temporal dynamics in gold. The third-order nonlinear susceptibility of the gold layer...... duration dependence of the third-order nonlinear susceptibility of gold is calculated in the broad range from tens of femtoseconds to tens of picoseconds using the two-temperature model of the free-electron temporal dynamics of gold, and shows the saturation of the thirdorder nonlinear susceptibility...

  3. Nonlinear phenomena in quantum thermoelectrics and heat

    Science.gov (United States)

    Sánchez, David; López, Rosa

    2016-12-01

    We review recent developments in nonlinear quantum transport through nanostructures and mesoscopic systems driven by thermal gradients or in combination with voltage biases. Low-dimensional conductors are excellent platforms for analyzing both the thermoelectric and heat dynamics beyond the linear response because, due to their small size, a small temperature difference applied across regions gives rise to large thermal biases. We offer a theoretical discussion based on the scattering approach to highlight the differences between the linear and the nonlinear regimes of transport. We discuss recent experiments on quantum dots and molecular junctions subjected to strong temperature differences. Theoretical predictions concerning the Kondo effect and heat rectification proposals are briefly examined. An important issue is the calculation of thermoelectric efficiencies including nonlinearities. Cross Seebeck effects and nonlinear spin filtering arise in superconductors and topological insulators, while mixed noises between charge and heat currents are also considered. Finally, we provide an outlook on the possible future directions of the field. xml:lang="fr"

  4. Hofstadter butterflies in nonlinear Harper lattices, and their optical realizations

    Energy Technology Data Exchange (ETDEWEB)

    Manela, Ofer; Segev, Mordechai [Department of Physics and Solid State Institute, Technion, Haifa 32000 (Israel); Christodoulides, Demetrios N [College of Optics/CREOL, University of Central Florida, FL 32816-2700 (United States); Kip, Detlef, E-mail: msegev@tx.technion.ac.i [Department of Electrical Engineering, Helmut Schmidt University, 22043 Hamburg (Germany)

    2010-05-15

    The ubiquitous Hofstadter butterfly describes a variety of systems characterized by incommensurable periodicities, ranging from Bloch electrons in magnetic fields and the quantum Hall effect to cold atoms in optical lattices and more. Here, we introduce nonlinearity into the underlying (Harper) model and study the nonlinear spectra and the corresponding extended eigenmodes of nonlinear quasiperiodic systems. We show that the spectra of the nonlinear eigenmodes form deformed versions of the Hofstadter butterfly and demonstrate that the modes can be classified into two families: nonlinear modes that are a 'continuation' of the linear modes of the system and new nonlinear modes that have no counterparts in the linear spectrum. Finally, we propose an optical realization of the linear and nonlinear Harper models in transversely modulated waveguide arrays, where these Hofstadter butterflies can be observed. This work is relevant to a variety of other branches of physics beyond optics, such as disorder-induced localization in ultracold bosonic gases, localization transition processes in disordered lattices, and more.

  5. Tunable Optical Sources and Synthetic Nonlinear Media: Growth and Characterization of Nonlinear Optical Materials

    Science.gov (United States)

    1992-02-13

    niobate and absolute measurements of nonlinear optical coefficients of six different commonly used nonlinear optical materials. The refractometry data for...applied radiation and is now an established technology for Nd:YAG lasers. Optical parametric oscillation and amplification provide a method of generating...continuously tunable output -3- The relative advantages of nonlinear optical frequency conversion compared to other methods for the generation of near

  6. Quantum Decoherence During Inflation from Gravitational Nonlinearities

    CERN Document Server

    Nelson, Elliot

    2016-01-01

    We study the inflationary quantum-to-classical transition for the adiabatic curvature perturbation $\\zeta$ due to quantum decoherence, focusing on the role played by squeezed-limit mode couplings. We evolve the quantum state $\\Psi$ in the Schr\\"odinger picture, for a generic cubic coupling to additional environment degrees of freedom. Focusing on the case of minimal gravitational interactions, we find the evolution of the reduced density matrix for a given long-wavelength fluctuation by tracing out the other (mostly shorterwavelength) modes of $\\zeta$ as an environment. We show that inflation produces phase oscillations in the wave functional $\\Psi[\\zeta(\\mathbf{x})]$, which suppress off-diagonal components of the reduced density matrix, leaving a diagonal mixture of different classical configurations. Gravitational nonlinearities thus provide a minimal mechanism for generating classical stochastic perturbations from inflation. We identify the time when decoherence occurs, which is delayed after horizon cross...

  7. Parameters estimation in quantum optics

    CERN Document Server

    D'Ariano, G M; Sacchi, M F; Paris, Matteo G. A.; Sacchi, Massimiliano F.

    2000-01-01

    We address several estimation problems in quantum optics by means of the maximum-likelihood principle. We consider Gaussian state estimation and the determination of the coupling parameters of quadratic Hamiltonians. Moreover, we analyze different schemes of phase-shift estimation. Finally, the absolute estimation of the quantum efficiency of both linear and avalanche photodetectors is studied. In all the considered applications, the Gaussian bound on statistical errors is attained with a few thousand data.

  8. Photonic Astronomy and Quantum Optics

    CERN Document Server

    Dravins, Dainis

    2015-01-01

    Quantum optics potentially offers an information channel from the Universe beyond the established ones of imaging and spectroscopy. All existing cameras and all spectrometers measure aspects of the first-order spatial and/or temporal coherence of light. However, light has additional degrees of freedom, manifest in the statistics of photon arrival times, or in the amount of photon orbital angular momentum. Such quantum-optical measures may carry information on how the light was created at the source, and whether it reached the observer directly or via some intermediate process. Astronomical quantum optics may help to clarify emission processes in natural laser sources and in the environments of compact objects, while high-speed photon-counting with digital signal handling enables multi-element and long-baseline versions of the intensity interferometer. Time resolutions of nanoseconds are required, as are large photon fluxes, making photonic astronomy very timely in an era of large telescopes.

  9. Optically simulated universal quantum computation

    Science.gov (United States)

    Francisco, D.; Ledesma, S.

    2008-04-01

    Recently, classical optics based systems to emulate quantum information processing have been proposed. The analogy is based on the possibility of encoding a quantum state of a system with a 2N-dimensional Hilbert space as an image in the input of an optical system. The probability amplitude of each state of a certain basis is associated with the complex amplitude of the electromagnetic field in a given slice of the laser wavefront. Temporal evolution is represented as the change of the complex amplitude of the field when the wavefront pass through a certain optical arrangement. Different modules that represent universal gates for quantum computation have been implemented. For instance, unitary operations acting on the qbits space (or U(2) gates) are represented by means of two phase plates, two spherical lenses and a phase grating in a typical image processing set up. In this work, we present CNOT gates which are emulated by means of a cube prism that splits a pair of adjacent rays incoming from the input image. As an example of application, we present an optical module that can be used to simulate the quantum teleportation process. We also show experimental results that illustrate the validity of the analogy. Although the experimental results obtained are promising and show the capability of the system for simulate the real quantum process, we must take into account that any classical simulation of quantum phenomena, has as fundamental limitation the impossibility of representing non local entanglement. In this classical context, quantum teleportation has only an illustrative interpretation.

  10. Effects of quantum noise on the nonlinear dynamics of a semiconductor laser subject to two spectrally filtered, time-delayed optical feedbacks

    Science.gov (United States)

    Suelzer, Joseph S.; Prasad, Awadhesh; Ghosh, Rupamanjari; Vemuri, Gautam

    2016-07-01

    We report on a theoretical and computational investigation of the complex dynamics that arise in a semiconductor laser that is subject to two external, time-delayed, filtered optical feedbacks with special attention to the effect of quantum noise. In particular, we focus on the dynamics of the instantaneous optical frequency (wavelength) and its behavior for a wide range of feedback strengths and filter parameters. In the case of two intermediate filter bandwidths, the most significant results are that in the presence of noise, the feedback strengths required for the onset of chaos in a period doubling route are higher than in the absence of noise. We find that the inclusion of noise changes the dominant frequency of the wavelength oscillations, and that certain attractors do not survive in the presence of noise for a range of filter parameters. The results are interpreted by use of a combination of phase portraits, rf spectra, and first return maps.

  11. Exciton-related nonlinear optical absorption and refractive index change in GaAs-Ga{sub 1-x}Al{sub x}As double quantum wells

    Energy Technology Data Exchange (ETDEWEB)

    Miranda, Guillermo L. [Fisica Teorica y Aplicada, Escuela de Ingenieria de Antioquia, A.A. 7516 Medellin (Colombia); Instituto de Fisica, Universidad de Antioquia, AA 1226 Medellin (Colombia); Mora-Ramos, Miguel E., E-mail: memora@uaem.mx [Fisica Teorica y Aplicada, Escuela de Ingenieria de Antioquia, A.A. 7516 Medellin (Colombia); Facultad de Ciencias, Universidad Autonoma del Estado de Morelos, Av. Universidad 1001, C.P. 62209 Cuernavaca, Morelos (Mexico); Instituto de Fisica, Universidad de Antioquia, AA 1226 Medellin (Colombia); Duque, Carlos A. [Instituto de Fisica, Universidad de Antioquia, AA 1226 Medellin (Colombia)

    2013-01-15

    In this work the variations of the exciton-related optical absorption and the change of the refractive index in a GaAs-(Ga,Al)As double quantum well as functions of the geometric parameters of the heterostructure are investigated. The variational method is applied within the framework of the parabolic band and effective mass approximations, in order to obtain the 1s-like exciton energy spectrum. The outcome for the related optical coefficients shows a quenched and redshifted light absorption as a result of the increment in the inner barrier and right-hand well widths, with the possibility of an enhancement of the excitonic contribution to the relative change in the refractive index.

  12. Linear and Nonlinear Plasmonics from Isotropic and Anisotropic Integrated Nanocomposites for Quantum Information Applications

    Science.gov (United States)

    2014-01-09

    nanoparticles (NPs) were added to luminescent porous silicon by drop casting. These NPs interact with this system by modifying its optical properties ...response by Au NPs in sapphire: Nonlinear optical response of Au metallic NPs, synthesized and embedded in sapphire by using ion implantation, as a...Linear and nonlinear plasmonics from isotropic and anisotropic integrated nanocomposites for quantum information applications. Jorge-Alejandro Reyes

  13. Quantum Optical Multiple Scattering

    DEFF Research Database (Denmark)

    Ott, Johan Raunkjær

    interference survives even after disorder averaging. The quantum interference manifests itself through increased photon correlations. Furthermore, the theoretical description of a measurement procedure is presented. In this work we relate the noise power spectrum of the total transmitted or reflected light......-state population and fluorescence spectrum, where we find cooperative effects in both the elastic and the inelastic spectra....

  14. Noise-free quantum optical frequency shifting driven by mechanics

    CERN Document Server

    Fan, Linran; Poot, Menno; Cheng, Risheng; Guo, Xiang; Han, Xu; Tang, Hong X

    2016-01-01

    The ability to manipulate single photons is of critical importance for fundamental quantum optics studies and practical implementations of quantum communications. While extraordinary progresses have been made in controlling spatial, temporal, spin and orbit angular momentum degrees of freedom, frequency-domain control of single photons so far relies on nonlinear optical effects, which have faced obstacles such as noise photons, narrow bandwidth and demanding optical filtering. Here we demonstrate the first integrated near-unity efficiency frequency manipulation of single photons, by stretching and compressing a waveguide at 8.3 billion cycles per second. Frequency shift up to 150 GHz at telecom wavelength is realized without measurable added noise and the preservation of quantum coherence is verified through quantum interference between twin photons of different colors. This single photon frequency control approach will be invaluable for increasing the channel capacity of quantum communications and compensati...

  15. Linear and nonlinear optical properties of a single dopant in strained AlAs/GaAs spherical core/shell quantum dots

    Science.gov (United States)

    El Haouari, M.; Talbi, A.; Feddi, E.; El Ghazi, H.; Oukerroum, A.; Dujardin, F.

    2017-01-01

    The hydrostatic pressure influence on the binding energy and on the optical properties (linear and third nonlinear) associated to the 1 s - 1 p intersubband transition of single dopant in a AlAs / GaAs spherical core/shell structure is investigated. The combined effects of the problem variables such as the core and shell sizes, the donor position in the structure and the pressure dependence of the physical parameters of the material have been analyzed. Our calculations are performed in the framework of the effective mass approximation and the energies are obtained by using a variational method. The results show that the linear and nonlinear parts of the absorption coefficient and the refractive index associated to the intersubband 1 s - 1 p transition undergo important changes. There are several interesting results to point out such as the shift of the absorption coefficients and refractive index to high values of photon energy. Another significant result is that the donor position considerably affects the optical properties and their corresponding amplitude.

  16. Metamaterials with tailored nonlinear optical response.

    Science.gov (United States)

    Husu, Hannu; Siikanen, Roope; Mäkitalo, Jouni; Lehtolahti, Joonas; Laukkanen, Janne; Kuittinen, Markku; Kauranen, Martti

    2012-02-08

    We demonstrate that the second-order nonlinear optical response of noncentrosymmetric metal nanoparticles (metamolecules) can be efficiently controlled by their mutual ordering in an array. Two samples with minor change in ordering have nonlinear responses differing by a factor of up to 50. The results arise from polarization-dependent plasmonic resonances modified by long-range coupling associated with metamolecular ordering. The approach opens new ways for tailoring the nonlinear responses of metamaterials and their tensorial properties.

  17. Nonlinear Sensing With Collective States of Ultracold Atoms in Optical Lattices

    Science.gov (United States)

    2015-04-02

    decimation algorithm , a method that takes into account quantum correlations. B.1. In collaboration with D. Blume and X.Y. Yin at Washington State...Office P.O. Box 12211 Research Triangle Park, NC 27709-2211 Nonlinear quantum sensing, quantum metrology, ultracold atoms, optical lattices REPORT...with applications to interaction-based quantum metrology, Physical Review A, (10 2014): 0. doi: 10.1103/PhysRevA.90.041602 Khan W Mahmud, Lei Jiang

  18. Nonlinear soliton matching between optical fibers

    DEFF Research Database (Denmark)

    Agger, Christian; Sørensen, Simon Toft; Thomsen, Carsten L.

    2011-01-01

    In this Letter, we propose a generic nonlinear coupling coefficient, η2 NL ¼ ηjγ=β2jfiber2=jγ=β2jfiber1, which gives a quantitative measure for the efficiency of nonlinear matching of optical fibers by describing how a fundamental soliton couples from one fiber into another. Specifically, we use η...

  19. All-optical switching in optically induced nonlinear waveguide couplers

    Energy Technology Data Exchange (ETDEWEB)

    Diebel, Falko, E-mail: falko.diebel@uni-muenster.de; Boguslawski, Martin; Rose, Patrick; Denz, Cornelia [Institut für Angewandte Physik and Center for Nonlinear Science (CeNoS), Westfälische Wilhelms-Universität Münster, 48149 Münster (Germany); Leykam, Daniel; Desyatnikov, Anton S. [Nonlinear Physics Centre, Research School of Physics and Engineering, The Australian National University, Canberra ACT 0200 (Australia)

    2014-06-30

    We experimentally demonstrate all-optical vortex switching in nonlinear coupled waveguide arrays optically induced in photorefractive media. Our technique is based on multiplexing of nondiffracting Bessel beams to induce various types of waveguide configurations. Using double- and quadruple-well potentials, we demonstrate precise control over the coupling strength between waveguides, the linear and nonlinear dynamics and symmetry-breaking bifurcations of guided light, and a power-controlled optical vortex switch.

  20. Development of Organic Nonlinear Optical Materials

    Science.gov (United States)

    1992-10-22

    10 SOVRCE Of FUNO#NG NUM#E*S DM J .j PROGRAM PR0jECT TA5. ~ *0. I1I TITLE &Vila* So.Ivety ClaUMC400NJ Development of Organic NonLinear Optical Materials (U...0102-LF-014-6603 UNCLASSIFIED (U) AFOSR Contract: F4962040-C 0097 FINAL REPORT Development of Organic Nonlinear Optical Materials by J. Sounnk IL

  1. Enhanced Kerr nonlinearity via quantum interference from spontaneous emission

    Energy Technology Data Exchange (ETDEWEB)

    Asadpour, S.H., E-mail: S.Hosein.Asadpour@gmail.com [Young Researchers Club, Bandar Anzali Branch, Islamic Azad University, Bandar Anzali (Iran, Islamic Republic of); Sahrai, M. [Research Institute for Applied Physics and Astronomy, University of Tabriz, Tabriz (Iran, Islamic Republic of); Soltani, A. [School of Engineering and Emerging Technologies, University of Tabriz, Tabriz (Iran, Islamic Republic of); Hamedi, H.R. [Research Institute for Applied Physics and Astronomy, University of Tabriz, Tabriz (Iran, Islamic Republic of)

    2012-01-02

    A novel atom configuration is proposed for a giant Kerr nonlinearity in zero linear and nonlinear probe absorption. It is shown that without coherent control field and just by quantum interference of spontaneous emission, a giant Kerr nonlinearity can be obtained. -- Highlights: ► The quantum interference from spontaneous emission is considered in a four-level medium. ► The giant Kerr nonlinearity in the zero linear and nonlinear absorption is obtained. ► The quantum interference effect on group velocity is then investigated.

  2. Optical realization of the dissipative quantum oscillator

    CERN Document Server

    Longhi, Stefano

    2016-01-01

    An optical realization of the damped quantum oscillator, based on transverse light dynamics in an optical resonator with slowly-moving mirrors, is theoretically suggested. The optical resonator setting provides a simple implementation of the time-dependent Caldirola-Kanai Hamiltonian of the dissipative quantum oscillator, and enables to visualize the effects of damped oscillations in the classical (ray optics) limit and wave packet collapse in the quantum (wave optics) regime.

  3. Optical resonators and quantum dots: An excursion into quantum optics, quantum information and photonics

    Science.gov (United States)

    Bianucci, Pablo

    Modern communications technology has encouraged an intimate connection between Semiconductor Physics and Optics, and this connection shows best in the combination of electron-confining structures with light-confining structures. Semiconductor quantum dots are systems engineered to trap electrons in a mesoscopic scale (the are composed of ≈ 10000 atoms), resulting in a behavior resembling that of atoms, but much richer. Optical microresonators are engineered to confine light, increasing its intensity and enabling a much stronger interaction with matter. Their combination opens a myriad of new directions, both in fundamental Physics and in possible applications. This dissertation explores both semiconductor quantum dots and microresonators, through experimental work done with semiconductor quantum dots and microsphere resonators spanning the fields of Quantum Optics, Quantum Information and Photonics; from quantum algorithms to polarization converters. Quantum Optics leads the way, allowing us to understand how to manipulate and measure quantum dots with light and to elucidate the interactions between them and microresonators. In the Quantum Information area, we present a detailed study of the feasibility of excitons in quantum dots to perform quantum computations, including an experimental demonstration of the single-qubit Deutsch-Jozsa algorithm performedin a single semiconductor quantum dot. Our studies in Photonics involve applications of microsphere resonators, which we have learned to fabricate and characterize. We present an elaborate description of the experimental techniques needed to study microspheres, including studies and proof of concept experiments on both ultra-sensitive microsphere sensors and whispering gallery mode polarization converters.

  4. Applications of quantum stochastic processes in quantum optics

    OpenAIRE

    Bouten, Luc

    2008-01-01

    These lecture notes provide an introduction to quantum filtering and its applications in quantum optics. We start with a brief introduction to quantum probability, focusing on the spectral theorem. Then we introduce the conditional expectation and quantum stochastic calculus. In the last part of the notes we discuss the filtering problem.

  5. Using supermodels in quantum optics

    Directory of Open Access Journals (Sweden)

    Garbers Nicole

    2006-01-01

    Full Text Available Starting from supersymmetric quantum mechanics and related supermodels within Schrödinger theory, we review the meaning of self-similar superpotentials which exhibit the spectrum of a geometric series. We construct special types of discretizations of the Schrödinger equation on time scales with particular symmetries. This discretization leads to the same type of point spectrum for the referred Schrödinger difference operator than in the self-similar superpotential case, hence exploiting an isospectrality situation. A discussion is opened on the question of how the considered energy sequence and its generalizations serve the understanding of coherent states in quantum optics.

  6. Completely integrable models of nonlinear optics

    Indian Academy of Sciences (India)

    Andrey I Maimistov

    2001-11-01

    The models of the nonlinear optics in which solitons appeared are considered. These models are of paramount importance in studies of nonlinear wave phenomena. The classical examples of phenomena of this kind are the self-focusing, self-induced transparency and parametric interaction of three waves. At present there are a number of theories based on completely integrable systems of equations, which are, both, generations of the original known models and new ones. The modified Korteweg-de Vries equation, the nonlinear Schrödinger equation, the derivative nonlinear Schrödinger equation, Sine–Gordon equation, the reduced Maxwell–Bloch equation, Hirota equation, the principal chiral field equations, and the equations of massive Thirring model are some soliton equations, which are usually to be found in nonlinear optics theory.

  7. Scale-invariant nonlinear optics in gases

    CERN Document Server

    Heyl, C M; Miranda, M; Louisy, M; Kovacs, K; Tosa, V; Balogh, E; Varjú, K; L'Huillier, A; Couairon, A; Arnold, C L

    2015-01-01

    Nonlinear optical methods are becoming ubiquitous in many areas of modern photonics. They are, however, often limited to a certain range of input parameters, such as pulse energy and average power, since restrictions arise from, for example, parasitic nonlinear effects, damage problems and geometrical considerations. Here, we show that many nonlinear optics phenomena in gaseous media are scale-invariant if spatial coordinates, gas density and laser pulse energy are scaled appropriately. We develop a general scaling model for (3+1)-dimensional wave equations, demonstrating the invariant scaling of nonlinear pulse propagation in gases. Our model is numerically applied to high-order harmonic generation and filamentation as well as experimentally verified using the example of pulse post-compression via filamentation. Our results provide a simple recipe for up-or downscaling of nonlinear processes in gases with numerous applications in many areas of science.

  8. Investigation of Optical Fibers for Nonlinear Optics.

    Science.gov (United States)

    1984-04-17

    Northwestern University, 1970. Experience Dr. Harrington has 13 years of research experi- ence in the area of optical properties of solids . Since joining...dynamics, and optical properties of solids . 34 34I ANTONIO C. PASTOR, Member of the Technical Staff, Optical Physics Department, Hughes Research

  9. Nonlinear Integrated Optical Waveguides in Chalcogenide Glasses

    Institute of Scientific and Technical Information of China (English)

    Yinlan; Ruan; Barry; Luther-Davies; Weitang; Li; Andrei; Rode; Marek; Samoc

    2003-01-01

    This paper reports on the study and measurement of the third order optical nonlinearity in bulk sulfide-based chalcogenide glasses; The fabrication process of the ultrafast laser deposited As-S-(Se)-based chalcogenide films and optical waveguides using two techniques: wet chemistry etching and plasma etching.

  10. Observation of optical-fiber Kerr nonlinearity at the single-photon level

    CERN Document Server

    Matsuda, Nobuyuki; Mitsumori, Yasuyoshi; Kosaka, Hideo; Edamatsu, Keiichi; 10.1038/nphoton.2008.292

    2012-01-01

    Optical fibers have been enabling numerous distinguished applications involving the operation and generation of light, such as soliton transmission, light amplification, all-optical switching and supercontinuum generation. The active function of optical fibers in the quantum regime is expected to be applicable to ultralow-power all-optical signal processing and quantum information processing. Here we demonstrate the first experimental observation of optical nonlinearity at the single-photon level in an optical fiber. Taking advantage of large nonlinearity and managed dispersion of a photonic crystal fiber, we have successfully measured very small (10^(-7) ~ 10^(-8)) conditional phase shifts induced by weak coherent pulses that contain one or less than one photon per pulse on average. In spite of its tininess, the phase shift was measurable using much (~10^6 times) stronger coherent probe pulses than the pump pulses. We discuss the feasibility of quantum information processing using optical fibers, taking into...

  11. Forbidden second order optical nonlinearity of graphene

    CERN Document Server

    Cheng, J L; Sipe, J E

    2016-01-01

    We present a practical scheme to separate the contributions of the electric quadrupole-like and the magnetic dipole-like effects to the forbidden second order optical nonlinear response of graphene, and give analytic expressions for the second order optical conductivities, calculated from the independent particle approximation, with relaxation described in a phenomenological way. We predict strong second order nonlinear effects, including second harmonic generation, photon drag, and difference frequency generation. We discuss in detail the controllablity of these responses by tuning the chemical potential, where the interband optical transitions play a dominant role.

  12. Nonlinear microstructured polymer optical fibres

    DEFF Research Database (Denmark)

    Frosz, Michael Henoch

    . The combination of a small core size and zero-dispersion wavelength at the operating wavelength of widely available femtosecond Ti:sapphire lasers led to an extensive research in supercontinuum generation and other nonlinear effects in PCFs. It is crucial for the efficiency of many nonlinear mechanisms...... that the pump laser wavelength is close to the zero-dispersion wavelength and that the core size is small. Recently, work in fabricating PCFs from materials other than silica has intensified. One of the advantages of using alternative materials can be a higher inherent material nonlinearity, which...... to accurately obtain a small core size while maintaining small structural variations during fibre drawing. This talk will give a presentation of how the mPOFs are fabricated and the route to obtaining nonlinear effects in them....

  13. Generation of non-classical optical fields by a beam splitter with second-order nonlinearity

    CERN Document Server

    Prakash, Hari

    2016-01-01

    We propose quantum-mechanical model of a beam splitter with second-order nonlinearity and show that non-classical features such as squeezing and sub-Poissonian photon statistics of optical fields can be generated in output fundamental and second harmonic modes when we mix coherent light beams via such a nonlinear beam splitter.

  14. Nonlinear optics with stationary pulses of light

    OpenAIRE

    Andre, A.; Bajcsy, M.; Zibrov, A. S.; Lukin, M. D.

    2004-01-01

    We show that the recently demonstrated technique for generating stationary pulses of light [Nature {\\bf 426}, 638 (2003)] can be extended to localize optical pulses in all three spatial dimensions in a resonant atomic medium. This method can be used to dramatically enhance the nonlinear interaction between weak optical pulses. In particular, we show that an efficient Kerr-like interaction between two pulses can be implemented as a sequence of several purely linear optical processes. The resul...

  15. Nonlinear optical properties of metal nanoparticle composites for optical applications

    Energy Technology Data Exchange (ETDEWEB)

    Takeda, Y. E-mail: takeda.yoshihiko@nims.go.jp; Kishimoto, N

    2003-05-01

    Optical absorption and nonlinear optical response were investigated for nanoparticle composites in amorphous SiO{sub 2} fabricated by negative Ta ion implantation at 60 keV. X-ray photoelectron spectroscopy was used to identify Ta and the oxide formation in the matrix. Optical absorption clearly indicated a surface plasmon peak at 2.2 eV and the peak resulted from formation of nanoparticles embedded in the matrix. The measured absorption was compared with calculated ones, evaluated by Maxwell-Garnett theory. Nonlinear absorption was measured with a pump-probe method using a femtosecond laser system. The pumping laser transiently bleached the surface plasmon band and lead to the nonlinearity. The transient response recovered in several picoseconds and behaved in terms of electron dynamics in metallic nanoparticles. The Ta nanoparticle composite is one of the promising candidates for nonlinear optical materials with good thermal stability.

  16. Quantum optical circulator controlled by a single chirally coupled atom

    Science.gov (United States)

    Scheucher, Michael; Hilico, Adèle; Will, Elisa; Volz, Jürgen; Rauschenbeutel, Arno

    2016-12-01

    Integrated nonreciprocal optical components, which have an inherent asymmetry between their forward and backward propagation direction, are key for routing signals in photonic circuits. Here, we demonstrate a fiber-integrated quantum optical circulator operated by a single atom. Its nonreciprocal behavior arises from the chiral interaction between the atom and the transversally confined light. We demonstrate that the internal quantum state of the atom controls the operation direction of the circulator and that it features a strongly nonlinear response at the single-photon level. This enables, for example, photon number–dependent routing and novel quantum simulation protocols. Furthermore, such a circulator can in principle be prepared in a coherent superposition of its operational states and may become a key element for quantum information processing in scalable integrated optical circuits.

  17. Nonlinear nanomechanical resonators for quantum optoelectromechanics

    CERN Document Server

    Rips, S; Hartmann, M J

    2012-01-01

    We present a scheme for enhancing the anharmonicity of nanomechanical resonators by subjecting them to inhomogenous electrostatic fields. We show that this approach enables access to a novel regime of optomechanics, where the nonlinearity per quanta of the mechanical motion becomes comparable to the linewidth of the optical cavities employed. In this "resolved nonlinearity regime" transitions between phonon Fock states of the mechanical resonator can be selectively addressed. As one application we show that our approach would allow to prepare stationary phonon Fock states in experimentally realistic devices. Such states are manifestly non-classical as they show pronounced negative Wigner functions. We calculate the mechanical steady state by tracing out the cavity modes in the weak optomechanical coupling limit and corroborate our results by a numerical analysis of the full dynamics including the cavity modes. Finally, we show how the negativity of the stationary states' Wigner function can be read off the ou...

  18. Optical rogue waves and soliton turbulence in nonlinear fibre optics

    DEFF Research Database (Denmark)

    Genty, G.; Dudley, J. M.; de Sterke, C. M.

    2009-01-01

    We examine optical rogue wave generation in nonlinear fibre propagation in terms of soliton turbulence. We show that higher-order dispersion is sufficient to generate localized rogue soliton structures, and Raman scattering effects are not required.......We examine optical rogue wave generation in nonlinear fibre propagation in terms of soliton turbulence. We show that higher-order dispersion is sufficient to generate localized rogue soliton structures, and Raman scattering effects are not required....

  19. Limiting effects of geometrical and optical nonlinearities on the squeezing in optomechanics

    Energy Technology Data Exchange (ETDEWEB)

    Djorwé, P. [Laboratory of Modelling and Simulation in Engineering, Biomimetics and Prototypes, Faculty of Science, University of Yaoundé I (Cameroon); Nana Engo, S.G., E-mail: nanaengo@gmail.com [Laboratory of Photonics, Faculty of Science, University of Ngaoundéré (Cameroon); Talla Mbé, J.H.; Woafo, P. [Laboratory of Modelling and Simulation in Engineering, Biomimetics and Prototypes, Faculty of Science, University of Yaoundé I (Cameroon)

    2013-08-01

    In recent experiments, the re-thermalization time of the mechanical resonator is stated as the limiting factor for quantum applications of optomechanical systems. To explain the origin of this limitation, an analytical nonlinear investigation supported by the recent successful experimental laser cooling parameters is carried out in this work. To this end, the effects of geometrical and the optical nonlinearities on the squeezing are studied and are in a good agreement with the experimental results. It appears that highly squeezed state are generated where these nonlinearities are minimized and that high nonlinearities are limiting factors to reach the quantum ground state.

  20. Nonlinear optical properties of semiconductor nanocrystals

    Science.gov (United States)

    Ricard, Gianpiero Banfi Vittorio Degiorgio Daniel

    1998-05-01

    This review is devoted to the description of recent experimental results concerning the nonlinear optical properties of semiconductor-doped glasses SDGs with particular emphasis on the regime in which the energy of the incident photon is smaller than the energy gap. A considerable theoretical and experimental effort has been devoted in the last 10years to the fundamental aspects of quantumconfined structures, which have properties somewhat intermediate between the bulk crystals and atoms or molecules. From this point of view, SDGs represent an easily available test system, and optical techniques have been a major diagnostic tool. Luminescence and absorption spectroscopy were extensively used to characterize the electronic states. The experiments aimed at the measurement of the real and imaginary parts of the third-order optical susceptibility of SDGs below the bandgap are described in some detail, and the results obtained with different techniques are compared. Besides the intrinsic fast nonlinearity due to bound electrons, SDGs may present a larger but much slower nonlinearity due to the free carriers generated by two-photon absorption. This implies that experiments have to be properly designed for separation of the two effects. In this article we stress the importance of a detailed structural characterization of the samples. Knowledge of the volume fraction occupied by the nanocrystals is necessary in order to derive from the experimental data the intrinsic nonlinearity and to compare it with the bulk nonlinearity. We discuss recent experiments in which the dependence of the intrinsic nonlinearity on the crystal size is derived by performing, on the samples, measurements of the real part and imaginary part of the nonlinear optical susceptibility and measurements of crystal size and volume fraction. Structural characterization is of interest also for a better understanding of the physical processes underlying the growth of crystallites in SDGs. The average size of

  1. Nonlinear optical model for strip plasmonic waveguides

    DEFF Research Database (Denmark)

    Lysenko, Oleg; Bache, Morten; Lavrinenko, Andrei

    2016-01-01

    This paper presents a theoretical model of nonlinear optical properties for strip plasmonic waveguides. The particular waveguides geometry that we investigate contains a gold core, adhesion layers, and silicon dioxide cladding. It is shown that the third-order susceptibility of the gold core...... significantly depends on the layer thickness and has the dominant contribution to the effective third-order susceptibility of the long-range plasmon polariton mode. This results in two nonlinear optical effects in plasmonic waveguides, which we experimentally observed and reported in [Opt. Lett. 41, 317 (2016......)]. The first effect is the nonlinear power saturation of the plasmonic mode, and the second effect is the spectral broadening of the plasmonic mode. Both nonlinear plasmonic effects can be used for practical applications and their appropriate model will be important for further developments in communication...

  2. BANDWIDTH OF QUANTUM OPTICAL COMMUNICATION SYSTEM

    Directory of Open Access Journals (Sweden)

    I. R. Gulakov

    2012-01-01

    Full Text Available Impact of registered optical radiation intensity, overvoltage, dimensions of photosensitive surface, structure of p-n junction and avalanche photodetectors dead time operating in the photon counting mode on quantum optical system capacity has been carried out in this investigation. As a result, the quantum optical system maximum capacity of 81 kbit/s has been obtained.

  3. Harmonic nanoparticles: noncentrosymmetric metal oxides for nonlinear optics

    Science.gov (United States)

    Rogov, Andrii; Mugnier, Yannick; Bonacina, Luigi

    2015-03-01

    The combination of nonlinear optics and nanotechnology is an extremely rich scientific domain yet widely unexplored. We present here a review of recent optical investigations on noncentrosymmetric oxide nanoparticles with a large {{χ }(2)} response, often referred to as harmonic nanoparticles (HNPs). HNPs feature a series of properties which distinguish them from other photonics nanoprobes (quantum dots, up-conversion nanoparticles, noble metal particles). HNPs emission is inherently nonlinear and based on the efficient generation of harmonics as opposed to fluorescence or surface plasmon scattering. In addition, the fully coherent signal emitted by HNPs together with their polarization sensitive response and absence of resonant interaction make them appealing for several applications ranging from multi-photon (infrared) microscopy and holography, to cell tracking and sensing.

  4. Strong electronic correlation effects in coherent multidimensional nonlinear optical spectroscopy.

    Science.gov (United States)

    Karadimitriou, M E; Kavousanaki, E G; Dani, K M; Fromer, N A; Perakis, I E

    2011-05-12

    We discuss a many-body theory of the coherent ultrafast nonlinear optical response of systems with a strongly correlated electronic ground state that responds unadiabatically to photoexcitation. We introduce a truncation of quantum kinetic density matrix equations of motion that does not rely on an expansion in terms of the interactions and thus applies to strongly correlated systems. For this we expand in terms of the optical field, separate out contributions to the time-evolved many-body state due to correlated and uncorrelated multiple optical transitions, and use "Hubbard operator" density matrices to describe the exact dynamics of the individual contributions within a subspace of strongly coupled states, including "pure dephasing". Our purpose is to develop a quantum mechanical tool capable of exploring how, by coherently photoexciting selected modes, one can trigger nonlinear dynamics of strongly coupled degrees of freedom. Such dynamics could lead to photoinduced phase transitions. We apply our theory to the nonlinear response of a two-dimensional electron gas (2DEG) in a magnetic field. We coherently photoexcite the two lowest Landau level (LL) excitations using three time-delayed optical pulses. We identify some striking temporal and spectral features due to dynamical coupling of the two LLs facilitated by inter-Landau-level magnetoplasmon and magnetoroton excitations and compare to three-pulse four-wave-mixing (FWM) experiments. We show that these features depend sensitively on the dynamics of four-particle correlations between an electron-hole pair and a magnetoplasmon/magnetoroton, reminiscent of exciton-exciton correlations in undoped semiconductors. Our results shed light into unexplored coherent dynamics and relaxation of the quantum Hall system (QHS) and can provide new insight into non-equilibrium co-operative phenomena in strongly correlated systems.

  5. Topological Quantum Optics in Two-Dimensional Atomic Arrays

    Science.gov (United States)

    Perczel, J.; Borregaard, J.; Chang, D. E.; Pichler, H.; Yelin, S. F.; Zoller, P.; Lukin, M. D.

    2017-07-01

    We demonstrate that two-dimensional atomic emitter arrays with subwavelength spacing constitute topologically protected quantum optical systems where the photon propagation is robust against large imperfections while losses associated with free space emission are strongly suppressed. Breaking time-reversal symmetry with a magnetic field results in gapped photonic bands with nontrivial Chern numbers and topologically protected, long-lived edge states. Due to the inherent nonlinearity of constituent emitters, such systems provide a platform for exploring quantum optical analogs of interacting topological systems.

  6. Non-reciprocal nonlinear optic induced transparency and frequency conversion on a chip

    CERN Document Server

    Guo, Xiang; Jung, Hojoong; Tang, Hong X

    2015-01-01

    Developments in photonic chips have spurred photon based classical and quantum information processing, attributing to the high stability and scalability of integrated photonic devices [1, 2]. Optical nonlinearity [3] is indispensable in these complex photonic circuits, because it allows for classical and quantum light sources, all-optical switch, modulation, and non-reciprocity in ambient environments. It is commonly known that nonlinear interactions are often greatly enhanced in the microcavities [4]. However, the manifestations of coherent photon-photon interaction in a cavity, analogous to the electromagnetically induced transparency [5], have never been reported on an integrated platform. Here, we present an experimental demonstration of the coherent photon-photon interaction induced by second order optical nonlinearity (\\chi^{(2)} ) on an aluminum nitride photonic chip. The non-reciprocal nonlinear optic induced transparency is demonstrated as a result of the coherent interference between photons with di...

  7. Experimental quantum forgery of quantum optical money

    Science.gov (United States)

    Bartkiewicz, Karol; Černoch, Antonín; Chimczak, Grzegorz; Lemr, Karel; Miranowicz, Adam; Nori, Franco

    2017-03-01

    Unknown quantum information cannot be perfectly copied (cloned). This statement is the bedrock of quantum technologies and quantum cryptography, including the seminal scheme of Wiesner's quantum money, which was the first quantum-cryptographic proposal. Surprisingly, to our knowledge, quantum money has not been tested experimentally yet. Here, we experimentally revisit the Wiesner idea, assuming a banknote to be an image encoded in the polarization states of single photons. We demonstrate that it is possible to use quantum states to prepare a banknote that cannot be ideally copied without making the owner aware of only unauthorized actions. We provide the security conditions for quantum money by investigating the physically-achievable limits on the fidelity of 1-to-2 copying of arbitrary sequences of qubits. These results can be applied as a security measure in quantum digital right management.

  8. Optical response in a laser-driven quantum pseudodot system

    Energy Technology Data Exchange (ETDEWEB)

    Kilic, D. Gul [Physics Department, Graduate School of Natural and Applied Sciences, Dokuz Eylül University, 35390 Izmir (Turkey); Sakiroglu, S., E-mail: serpil.sakiroglu@deu.edu.tr [Physics Department, Faculty of Science, Dokuz Eylül University, 35390 Izmir (Turkey); Ungan, F.; Yesilgul, U. [Department of Optical Engineering, Faculty of Technology, Cumhuriyet University, 58140 Sivas (Turkey); Kasapoglu, E. [Physics Department, Faculty of Science, Cumhuriyet University, 58140 Sivas (Turkey); Sari, H. [Department of Primary Education, Faculty of Education, Cumhuriyet University, 58140 Sivas (Turkey); Sokmen, I. [Physics Department, Faculty of Science, Dokuz Eylül University, 35390 Izmir (Turkey)

    2017-03-15

    We investigate theoretically the intense laser-induced optical absorption coefficients and refractive index changes in a two-dimensional quantum pseudodot system under an uniform magnetic field. The effects of non-resonant, monochromatic intense laser field upon the system are treated within the framework of high-frequency Floquet approach in which the system is supposed to be governed by a laser-dressed potential. Linear and nonlinear absorption coefficients and relative changes in the refractive index are obtained by means of the compact-density matrix approach and iterative method. The results of numerical calculations for a typical GaAs quantum dot reveal that the optical response depends strongly on the magnitude of external magnetic field and characteristic parameters of the confinement potential. Moreover, we have demonstrated that the intense laser field modifies the confinement and thereby causes remarkable changes in the linear and nonlinear optical properties of the system.

  9. Tunable nanowire nonlinear optical probe

    Energy Technology Data Exchange (ETDEWEB)

    Nakayama, Yuri; Pauzauskie, Peter J.; Radenovic, Aleksandra; Onorato, Robert M.; Saykally, Richard J.; Liphardt, Jan; Yang, Peidong

    2008-02-18

    One crucial challenge for subwavelength optics has been thedevelopment of a tunable source of coherent laser radiation for use inthe physical, information, and biological sciences that is stable at roomtemperature and physiological conditions. Current advanced near-fieldimaging techniques using fiber-optic scattering probes1,2 have alreadyachieved spatial resolution down to the 20-nm range. Recently reportedfar-field approaches for optical microscopy, including stimulatedemission depletion (STED)3, structured illumination4, and photoactivatedlocalization microscopy (PALM)5, have also enabled impressive,theoretically-unlimited spatial resolution of fluorescent biomolecularcomplexes. Previous work with laser tweezers6-8 has suggested the promiseof using optical traps to create novel spatial probes and sensors.Inorganic nanowires have diameters substantially below the wavelength ofvisible light and have unique electronic and optical properties9,10 thatmake them prime candidates for subwavelength laser and imagingtechnology. Here we report the development of an electrode-free,continuously-tunable coherent visible light source compatible withphysiological environments, from individual potassium niobate (KNbO3)nanowires. These wires exhibit efficient second harmonic generation(SHG), and act as frequency converters, allowing the local synthesis of awide range of colors via sum and difference frequency generation (SFG,DFG). We use this tunable nanometric light source to implement a novelform of subwavelength microscopy, in which an infrared (IR) laser is usedto optically trap and scan a nanowire over a sample, suggesting a widerange of potential applications in physics, chemistry, materials science,and biology.

  10. Strongly Correlated Quantum Walks in Optical Lattices

    OpenAIRE

    Preiss, Philipp M.; Ma, Ruichao; Tai, M. Eric; Lukin, Alexander; Rispoli, Matthew; Zupancic, Philip; Lahini, Yoav; Islam, Rajibul; Greiner, Markus

    2014-01-01

    Full control over the dynamics of interacting, indistinguishable quantum particles is an important prerequisite for the experimental study of strongly correlated quantum matter and the implementation of high-fidelity quantum information processing. Here we demonstrate such control over the quantum walk - the quantum mechanical analogue of the classical random walk - in the strong interaction regime. Using interacting bosonic atoms in an optical lattice, we directly observe fundamental effects...

  11. Towards multimodal nonlinear optical tomography - experimental methodology

    Science.gov (United States)

    Vogler, N.; Medyukhina, A.; Latka, I.; Kemper, S.; Böhm, M.; Dietzek, B.; Popp, J.

    2011-08-01

    All-optical microspectroscopic and tomographic tools reveal great potential for clinical dermatologic diagnostics, i.e., investigation of human skin and skin diseases. While optical-coherence tomography has been complemented by two-photon fluorescence tomography and second-harmonic generation tomography, a joint study of various nonlinear optical microspectroscopies, i.e., application of the recently developed multimodal imaging approach, to sizable human-tissue samples has not been evaluated up to now. Here, we present such multimodal approach combining different nonlinear optical contrast mechanisms for imaging, namely two-photon excited fluorescence (TPF), second-harmonic generation (SHG), and coherent anti-Stokes Raman scattering (CARS) into a joint microscopic experiment. We show the potential of imaging large skin areas and discuss the information obtained in a case study comparing normal skin and keloid tissue.

  12. Femtojoule-Scale All-Optical Latching and Modulation via Cavity Nonlinear Optics

    Science.gov (United States)

    Kwon, Yeong-Dae; Armen, Michael A.; Mabuchi, Hideo

    2013-11-01

    We experimentally characterize Hopf bifurcation phenomena at femtojoule energy scales in a multiatom cavity quantum electrodynamical (cavity QED) system and demonstrate how such behaviors can be exploited in the design of all-optical memory and modulation devices. The data are analyzed by using a semiclassical model that explicitly treats heterogeneous coupling of atoms to the cavity mode. Our results highlight the interest of cavity QED systems for ultralow power photonic signal processing as well as for fundamental studies of mesoscopic nonlinear dynamics.

  13. Investigating macroscopic quantum superpositions and the quantum-to-classical transition by optical parametric amplification

    CERN Document Server

    De Martini, Francesco

    2012-01-01

    The present work reports on an extended research endeavor focused on the theoretical and experimental realization of a macroscopic quantum superposition (MQS) made up with photons. As it is well known, this intriguing, fundamental quantum condition is at the core of a famous argument conceived by Erwin Schroedinger, back in 1935. The main experimental challenge to the actual realization of this object resides generally on the unavoidable and uncontrolled interactions with the environment, i.e. the decoherence leading to the cancellation of any evidence of the quantum features associated with the macroscopic system. The present scheme is based on a nonlinear process, the "quantum injected optical parametric amplification", that maps by a linearized cloning process the quantum coherence of a single - particle state, i.e. a Micro - qubit, into a Macro - qubit, consisting in a large number M of photons in quantum superposition. Since the adopted scheme was found resilient to decoherence, the MQS\\ demonstration wa...

  14. Few-photon Non-linearities in Nanophotonic Devices for Quantum Information Technology

    DEFF Research Database (Denmark)

    Nysteen, Anders

    In this thesis we investigate few-photon non-linearities in all-optical, on-chip circuits, and we discuss their possible applications in devices of interest for quantum information technology, such as conditional two-photon gates and single-photon sources. In order to propose efficient devices...

  15. Interaction-induced effects in the nonlinear coherent response of quantum-well excitons

    DEFF Research Database (Denmark)

    Wagner, Hans Peter; Schätz, A.; Langbein, Wolfgang Werner;

    1999-01-01

    Interaction-induced processes are studied using the third-order nonlinear polarization created in polarization-dependent four-wave-mixing experiments (FWM) on a ZnSe single quantum well. We discuss their influence by a comparison of the experimental FWM with calculations based on extended optical...

  16. Quantum Computations with Transverse Modes of an Optical Field Propagating in Waveguides

    Institute of Scientific and Technical Information of China (English)

    符建; 唐少芳

    2003-01-01

    A fully optical method to perform quantum computation with transverse modes of the optical field propagating in waveguide is proposed by supplying the prescriptions for a universal set of quantum gates. The proposal for quantum computation is based on implementing a quantum bit with two normal modes of multi-mode waveguides. The proposed C-NOT gate has the potential of being more compact and easily realized than some optical implementations, since it is based on planar lightwave circuit technology and can be constructed by using Mach-Zehnder interferometer having semiconductor optical amplifiers with very large refractive nonlinearity in its arms.

  17. Recent Issues on Nonlinear Effects in Optical Fibers

    Institute of Scientific and Technical Information of China (English)

    Takashi; Inoue; Osamu; Aso; Shu; Namiki

    2003-01-01

    This talk will discuss the types of optical signal degradation due to fiber nonlinearity and review recently invented fibers for suppressing the effects. It also introduces efficiency of highly nonlinear fibers and their applications to nonlinear signal processing.

  18. Nonlinearities in the quantum measurement process of superconducting qubits

    Energy Technology Data Exchange (ETDEWEB)

    Serban, Ioana

    2008-05-15

    The work described in this thesis focuses on the investigation of decoherence and measurement backaction, on the theoretical description of measurement schemes and their improvement. The study presented here is centered around quantum computing implementations using superconducting devices and most important, the Josephson effect. The measured system is invariantly a qubit, i. e. a two-level system. The objective is to study detectors with increasing nonlinearity, e. g. coupling of the qubit to the frequency a driven oscillator, or to the bifurcation amplifier, to determine the performance and backaction of the detector on the measured system and to investigate the importance of a strong qubit-detector coupling for the achievement of a quantum non-demolition type of detection. The first part gives a very basic introduction to quantum information, briefly reviews some of the most promising physical implementations of a quantum computer before focusing on the superconducting devices. The second part presents a series of studies of different qubit measurements, describing the backaction of the measurement onto the measured system and the internal dynamics of the detector. Methodology adapted from quantum optics and chemical physics (master equations, phase-space analysis etc.) combined with the representation of a complex environment yielded a tool capable of describing a nonlinear, non-Markovian environment, which couples arbitrarily strongly to the measured system. This is described in chapter 3. Chapter 4 focuses on the backaction on the qubit and presents novel insights into the qubit dephasing in the strong coupling regime. Chapter 5 uses basically the same system and technical tools to explore the potential of a fast, strong, indirect measurement, and determine how close such a detection would ideally come to the quantum non-demolition regime. Chapter 6 focuses on the internal dynamics of a strongly driven Josephson junction. The analytical results are based on

  19. Nonlinear microstructured polymer optical fibres

    DEFF Research Database (Denmark)

    Frosz, Michael Henoch

    is potentially the case for microstructured polymer optical fibres (mPOFs). Another advantage is that polymer materials have a higher biocompatibility than silica, meaning that it is easier to bond certain types of biosensor materials to a polymer surface than to silica. As with silica PCFs, it is difficult...

  20. Quantum mechanical design of efficient second-order nonlinear optical materials based on heteroaromatic imido-substituted hexamolybdates: first theoretical framework of POM-based heterocyclic aromatic rings.

    Science.gov (United States)

    Janjua, Muhammad Ramzan Saeed Ashraf

    2012-11-05

    This work was inspired by a previous report (Janjua et al. J. Phys. Chem. A 2009, 113, 3576-3587) in which the nonlinear-optical (NLO) response strikingly improved with an increase in the conjugation path of the ligand and the nature of hexamolybdates (polyoxometalates, POMs) was changed into a donor by altering the direction of charge transfer with a second aromatic ring. Herein, the first theoretical framework of POM-based heteroaromatic rings is found to be another class of excellent NLO materials having double heteroaromatic rings. First hyperpolarizabilities of a large number of push-pull-substituted conjugated systems with heteroaromatic rings have been calculated. The β components were computed at the density functional theory (DFT) level (BP86 geometry optimizations and LB94 time-dependent DFT). The largest β values are obtained with a donor (hexamolybdates) on the benzene ring and an acceptor (-NO(2)) on pyrrole, thiophene, and furan rings. The pyrrole imido-substituted hexamolybdate (system 1c) has a considerably large first hyperpolarizability, 339.00 × 10(-30) esu, and it is larger than that of (arylimido)hexamolybdate, calculated as 0.302 × 10(-30) esu (reference system 1), because of the double aromatic rings in the heteroaromatic imido-substituted hexamolybdates. The heteroaromatic rings act as a conjugation bridge between the electron acceptor (-NO(2)) and donor (polyanion). The introduction of an electron donor into heteroaromatic rings significantly enhances the first hyperpolarizabilities because the electron-donating ability is substantially enhanced when the electron donor is attached to the heterocyclic aromatic rings. Interposing five-membered auxiliary fragments between strong donor (polyanion) or acceptor (-NO(2)) groups results in a large computed second-order NLO response. The present investigation provides important insight into the NLO properties of (heteroaromatic) imido-substituted hexamolybdate derivatives because these compounds

  1. Localized Turing patterns in nonlinear optical cavities

    Science.gov (United States)

    Kozyreff, G.

    2012-05-01

    The subcritical Turing instability is studied in two classes of models for laser-driven nonlinear optical cavities. In the first class of models, the nonlinearity is purely absorptive, with arbitrary intensity-dependent losses. In the second class, the refractive index is real and is an arbitrary function of the intracavity intensity. Through a weakly nonlinear analysis, a Ginzburg-Landau equation with quintic nonlinearity is derived. Thus, the Maxwell curve, which marks the existence of localized patterns in parameter space, is determined. In the particular case of the Lugiato-Lefever model, the analysis is continued to seventh order, yielding a refined formula for the Maxwell curve and the theoretical curve is compared with recent numerical simulation by Gomila et al. [D. Gomila, A. Scroggie, W. Firth, Bifurcation structure of dissipative solitons, Physica D 227 (2007) 70-77.

  2. Experimental investigation of nonlinear optical properties of Ag nanoparticles: Effects of size quantization

    Science.gov (United States)

    Sato, Rodrigo; Ohnuma, Masato; Oyoshi, Keiji; Takeda, Yoshihiko

    2014-09-01

    The effects of size quantization on the nonlinear optical response of Ag nanoparticles are experimentally studied by spectroscopic ellipsometry and femtosecond spectroscopic pump-and-probe techniques. In the vicinity of a localized surface-plasmon resonance (2.0-3.5 eV), we have investigated the optical nonlinearity of Ag particles embedded in silica glass for particle diameters ranging from 3.0 to 16 nm. The intrinsic third-order optical susceptibility χm(3) of Ag particles exhibited significant spectral and size dependences. These results are explained as quantum and dielectric confinements and are compared to the results of theoretical quantum finite-size effects calculation for metallic particles. In light of these results, we discuss the contribution of interband transitions to the size dependence of χm(3). Quantum size effects lead to an increase in nonlinearity in small Ag particles.

  3. Infiltrated microstructured fibers as tunable and nonlinear optical devices

    DEFF Research Database (Denmark)

    Rosberg, Christian Romer; Bennet, Francis; Neshev, Dragomir N.;

    We study the light guiding properties of microstructured optical fibers infiltrated with nonlinear liquids and demonstrate their applicability for spatial beam control in novel type tunable and nonlinear optical devices....

  4. Laser and nonlinear optical materials: SPIE volume 681

    Energy Technology Data Exchange (ETDEWEB)

    De Shazer, L.G.

    1987-01-01

    This book contains papers arranged under the following session headings: Nonlinear optical crystals; Laser host crystals; Electro-optic and magneto-optic materials; and Characterization of optical materials.

  5. Nonlinear optical studies of relaxation in semiconductor microstructures

    Science.gov (United States)

    Remillard, Jeffrey Thomas

    1990-11-01

    Exposing a semiconductor to optical radiation near the fundamental band gap results in the creation of populations or elementary excitations including electrons, holes, and excitons, and also results in the creation of a superposition state between the ground and excited state of the solid. The relaxation of optically generated excitons and carriers in semiconductor microstructures was studied using four wave mixing (FWM) spectroscopy. The systems studied include CdSSe microcrystallite doped glasses and GaA/AlGaAs multiple quantum well structures (MQWS). First, the nonlinear optical response of simple two level systems is examined in order to provide insight into the types of line shapes expected from semiconductors. It is shown that the line shape is strongly dependent on how the system is coupled to the reservoir and the consequences of coupling to a reservoir are examined in a FWM measurement made in atomic sodium. The first semiconductor system studied is CdSSe microcrystallite doped glass. This system is shown to have a very slow component to the nonlinear response which has an optical intensity dependence and temperature dependence which suggests that the FWM response in these materials is trap mediated. Room temperature FWM measurements in GaAs MQWS enables the measurement of the carrier recombination time and the ambipolar diffusion coefficient. Using the technique of correlated optical fields, a slow component to the nonlinear response was measured showing an interference profile which suggests a possible shift of the exciton resonance due to the optically generated carriers. At low temperatures, measurements of the exciton line shape and relaxation time were made and evidence for exciton spectral diffusion was found. The low temperature line shapes can be qualitatively reproduced using Modified Optical Bloch equations which include the effects of spectral diffusion.

  6. Nonlinear compression of optical solitons

    Indian Academy of Sciences (India)

    M N Vinoj; V C Kuriakose

    2001-11-01

    In this paper, we consider nonlinear Schrödinger (NLS) equations, both in the anomalous and normal dispersive regimes, which govern the propagation of a single field in a fiber medium with phase modulation and fibre gain (or loss). The integrability conditions are arrived from linear eigen value problem. The variable transformations which connect the integrable form of modified NLS equations are presented. We succeed in Hirota bilinearzing the equations and on solving, exact bright and dark soliton solutions are obtained. From the results, we show that the soliton is alive, i.e. pulse area can be conserved by the inclusion of gain (or loss) and phase modulation effects.

  7. Giant kerr nonlinearity, controlled entangled photons and polarization phase gates in coupled quantum-well structures.

    Science.gov (United States)

    Zhu, Chengjie; Huang, Guoxiang

    2011-11-07

    We study linear and nonlinear propagations of probe and signal pulses in a multiple quantum-well structure with a four-level, double Λ-type configuration. We show that slow, mutually matched group velocities and giant Kerr nonlinearity of the probe and the signal pulses may be achieved with nearly vanishing optical absorption. Based on these properties we demonstrate that two-qubit quantum polarization phase gates can be constructed and highly entangled photon pairs may be produced. In addition, we show that coupled slow-light soliton pairs with very low generation power can be realized in the system.

  8. Nonlinear excitation kinetics of biased quantum wells. Coherent dynamical screening effect

    DEFF Research Database (Denmark)

    Turchinovich, Dmitry; Jepsen, Peter Uhd

    2006-01-01

    In this paper we describe a strongly nonlinear process of ultrafast photoexcitation of a biased quantum well. This process is governed by coherent dynamical screening, where the instantaneously polarized photoexcited carriers screen initial bias field. This results in a dynamic modification...... of the bandstructure of the quantum well, which is totally coherent with the temporal intensity distribution of the excitation laser pulse. We developed a time-resolved theoretical model of coherent dynamical screening, which predicts interesting fundamental consequences, such as nonlinear absorption and ultra......-broadband THz emission. The results of our THz and optical experiments are in good agreement with the theoretical model....

  9. NONLINEAR OPTICS: Nonlinear optical processes in planar waveguides and excitation of surface polaritons

    Science.gov (United States)

    Yashkir, O. V.; Yashkir, Yu N.

    1987-11-01

    An investigation is made of nonlinear optical interaction of light propagating in a planar waveguide with surface polaritons. Reduced wave equations for the amplitudes of the waveguide modes and surface polaritons are used to study the characteristics of generation of surface polaritons of difference frequency, parametric frequency up-conversion of the polaritons, and stimulated Raman scattering by the polaritons. An analysis is made of the characteristic properties of the investigated nonlinear optical processes.

  10. Optimal state discrimination and unstructured search in nonlinear quantum mechanics

    Science.gov (United States)

    Childs, Andrew M.; Young, Joshua

    2016-02-01

    Nonlinear variants of quantum mechanics can solve tasks that are impossible in standard quantum theory, such as perfectly distinguishing nonorthogonal states. Here we derive the optimal protocol for distinguishing two states of a qubit using the Gross-Pitaevskii equation, a model of nonlinear quantum mechanics that arises as an effective description of Bose-Einstein condensates. Using this protocol, we present an algorithm for unstructured search in the Gross-Pitaevskii model, obtaining an exponential improvement over a previous algorithm of Meyer and Wong. This result establishes a limitation on the effectiveness of the Gross-Pitaevskii approximation. More generally, we demonstrate similar behavior under a family of related nonlinearities, giving evidence that the ability to quickly discriminate nonorthogonal states and thereby solve unstructured search is a generic feature of nonlinear quantum mechanics.

  11. Polarization-Sensitive Quantum Optical Coherence Tomography: Experiment

    CERN Document Server

    Booth, Mark C; Teich, Malvin Carl

    2010-01-01

    Polarization-sensitive quantum optical coherence tomography (PS-QOCT) makes use of a Type-II twin-photon light source for carrying out optical sectioning with polarization sensitivity. A BBO nonlinear optical crystal pumped by a Ti:sapphire psec-pulsed laser is used to confirm the theoretical underpinnings of this imaging paradigm. PS-QOCT offers even-order dispersion cancellation with simultaneous access to the group-velocity dispersion characteristics of the interstitial medium between the reflecting surfaces of the sample.

  12. Quantum computation architecture using optical tweezers

    DEFF Research Database (Denmark)

    Weitenberg, Christof; Kuhr, Stefan; Mølmer, Klaus;

    2011-01-01

    We present a complete architecture for scalable quantum computation with ultracold atoms in optical lattices using optical tweezers focused to the size of a lattice spacing. We discuss three different two-qubit gates based on local collisional interactions. The gates between arbitrary qubits...... quantum computing....

  13. Coherent analysis of quantum optical sideband modes

    CERN Document Server

    Huntington, E H; Robilliard, C; Ralph, T C

    2005-01-01

    We demonstrate a device that allows for the coherent analysis of a pair of optical frequency sidebands in an arbitrary basis. We show that our device is quantum noise limited and hence applications for this scheme may be found in discrete and continuous variable optical quantum information experiments.

  14. Anisotropic and nonlinear optical waveguides

    CERN Document Server

    Someda, CG

    1992-01-01

    Dielectric optical waveguides have been investigated for more than two decades. In the last ten years they have had the unique position of being simultaneously the backbone of a very practical and fully developed technology, as well as an extremely exciting area of basic, forefront research. Existing waveguides can be divided into two sets: one consisting of waveguides which are already in practical use, and the second of those which are still at the laboratory stage of their evolution. This book is divided into two separate parts: the first dealing with anisotropic waveguides, an

  15. Virial Theorem for a Class of Quantum Nonlinear Harmonic Oscillators

    Institute of Scientific and Technical Information of China (English)

    王雪红; 郭军义; 李艳

    2012-01-01

    In this paper,the Virial Theorem based on a class of quantum nonlinear harmonic oscillators is presented.This relationship has to do with parameter λ and ?/?λ,where the λ is a real number.When λ=0,the nonlinear harmonic oscillator naturally reduces to the usual quantum linear harmonic oscillator,and the Virial Theorem also reduces to the usual Virial Theorem.

  16. Fresnel-Transform's Quantum Correspondence and Quantum Optical ABCD Law

    Institute of Scientific and Technical Information of China (English)

    FAN Hong-Yi; HU Li-Yun

    2007-01-01

    @@ Corresponding to the Fresnel transform there exists a unitary operator in quantum optics theory, which could be known the Fresnel operator (FO). We show that the multiplication rule of the FO naturally leads to the quantum optical ABCD law. The canonical operator methods as mapping of ray-transfer ABCD matrix is explicitly shown by the normally ordered expansion of the FO through the coherent state representation and the technique of integration within an ordered product of operators. We show that time evolution of the damping oscillator embodies the quantum optical ABCD law.

  17. Bifurcation-based adiabatic quantum computation with a nonlinear oscillator network.

    Science.gov (United States)

    Goto, Hayato

    2016-02-22

    The dynamics of nonlinear systems qualitatively change depending on their parameters, which is called bifurcation. A quantum-mechanical nonlinear oscillator can yield a quantum superposition of two oscillation states, known as a Schrödinger cat state, via quantum adiabatic evolution through its bifurcation point. Here we propose a quantum computer comprising such quantum nonlinear oscillators, instead of quantum bits, to solve hard combinatorial optimization problems. The nonlinear oscillator network finds optimal solutions via quantum adiabatic evolution, where nonlinear terms are increased slowly, in contrast to conventional adiabatic quantum computation or quantum annealing, where quantum fluctuation terms are decreased slowly. As a result of numerical simulations, it is concluded that quantum superposition and quantum fluctuation work effectively to find optimal solutions. It is also notable that the present computer is analogous to neural computers, which are also networks of nonlinear components. Thus, the present scheme will open new possibilities for quantum computation, nonlinear science, and artificial intelligence.

  18. Bifurcation-based adiabatic quantum computation with a nonlinear oscillator network

    Science.gov (United States)

    Goto, Hayato

    2016-02-01

    The dynamics of nonlinear systems qualitatively change depending on their parameters, which is called bifurcation. A quantum-mechanical nonlinear oscillator can yield a quantum superposition of two oscillation states, known as a Schrödinger cat state, via quantum adiabatic evolution through its bifurcation point. Here we propose a quantum computer comprising such quantum nonlinear oscillators, instead of quantum bits, to solve hard combinatorial optimization problems. The nonlinear oscillator network finds optimal solutions via quantum adiabatic evolution, where nonlinear terms are increased slowly, in contrast to conventional adiabatic quantum computation or quantum annealing, where quantum fluctuation terms are decreased slowly. As a result of numerical simulations, it is concluded that quantum superposition and quantum fluctuation work effectively to find optimal solutions. It is also notable that the present computer is analogous to neural computers, which are also networks of nonlinear components. Thus, the present scheme will open new possibilities for quantum computation, nonlinear science, and artificial intelligence.

  19. Extreme nonlinear optics and laser damage

    Science.gov (United States)

    Maldutis, Evaldas

    2010-11-01

    The study of laser induced damage threshold caused by series of identical laser pulses (LID-T-N) on gamma radiation resistant glasses and their analogs is performed applying know-how ultra stable laser radiation. The presented results and analysis of earlier received results show that nonlinear optical phenomena in extreme conditions of interaction are different from the traditional nonlinear optical processes, because they depend not only on intensity of electromagnetic field of laser radiation, but also on the pulse number in series of identical laser pulses. This range of laser intensities is not wide; it is different for each material and determines the range of Extreme Nonlinear Optics. The dependence of LID-T-N on pulse number N for different kinds of high quality transparent glasses was observed. The study of dynamics of these processes (i.e. the study of dependence on N) at different intensities in series of incident laser pulses provides new information about properties of the materials useful for studying laser damage fundamentals and their application. The expectation that gamma radiation resistant glasses could give useful information for technology of resistant optics for high power lasers has not proved. The received results well correspond with the earlier proposed model of laser damage.

  20. Rigorous theory of molecular orientational nonlinear optics

    Directory of Open Access Journals (Sweden)

    Chong Hoon Kwak

    2015-01-01

    Full Text Available Classical statistical mechanics of the molecular optics theory proposed by Buckingham [A. D. Buckingham and J. A. Pople, Proc. Phys. Soc. A 68, 905 (1955] has been extended to describe the field induced molecular orientational polarization effects on nonlinear optics. In this paper, we present the generalized molecular orientational nonlinear optical processes (MONLO through the calculation of the classical orientational averaging using the Boltzmann type time-averaged orientational interaction energy in the randomly oriented molecular system under the influence of applied electric fields. The focal points of the calculation are (1 the derivation of rigorous tensorial components of the effective molecular hyperpolarizabilities, (2 the molecular orientational polarizations and the electronic polarizations including the well-known third-order dc polarization, dc electric field induced Kerr effect (dc Kerr effect, optical Kerr effect (OKE, dc electric field induced second harmonic generation (EFISH, degenerate four wave mixing (DFWM and third harmonic generation (THG. We also present some of the new predictive MONLO processes. For second-order MONLO, second-order optical rectification (SOR, Pockels effect and difference frequency generation (DFG are described in terms of the anisotropic coefficients of first hyperpolarizability. And, for third-order MONLO, third-order optical rectification (TOR, dc electric field induced difference frequency generation (EFIDFG and pump-probe transmission are presented.

  1. Nonlinear Mixing in Optical Multicarrier Systems

    Science.gov (United States)

    Hameed, Mahmood Abdul

    Although optical fiber has a vast spectral bandwidth, efficient use of this bandwidth is still important in order to meet the ever increased capacity demand of optical networks. In addition to wavelength division multiplexing, it is possible to partition multiple low-rate subcarriers into each high speed wavelength channel. Multicarrier systems not only ensure efficient use of optical and electrical components, but also tolerate transmission impairments. The purpose of this research is to understand the impact of mixing among subcarriers in Radio-Over-Fiber (RoF) and high speed optical transmission systems, and experimentally demonstrate techniques to minimize this impact. We also analyze impact of clipping and quantization on multicarrier signals and compare bandwidth efficiency of two popular multiplexing techniques, namely, orthogonal frequency division multiplexing (OFDM) and Nyquist modulation. For an OFDM-RoF system, we present a novel technique that minimizes the RF domain signal-signal beat interference (SSBI), relaxes the phase noise limit on the RF carrier, realizes the full potential of optical heterodyne-based RF carrier generation, and increases the performance-to-cost ratio of RoF systems. We demonstrate a RoF network that shares the same RF carrier for both downlink and uplink, avoiding the need of an additional RF oscillator in the customer unit. For multi-carrier optical transmission, we first experimentally compare performance degradations of coherent optical OFDM and single-carrier Nyquist pulse modulated systems in a nonlinear environment. We then experimentally evaluate SSBI compensation techniques in the presence of semiconductor optical amplifier (SOA) induced nonlinearities for a multicarrier optical system with direct detection. We show that SSBI contamination can be significantly reduced from the data signal when the carrier-to-signal power ratio is sufficiently low.

  2. Optically nonlinear Langmuir Blodgett films

    CERN Document Server

    Amiri, M A

    2003-01-01

    A series of novel amphiphilic molecules plus a new class of chevron-shaped materials, without aliphatic tails, were designed, synthesised and non-centrosymmetrically aligned by the Langmuir-Blodgett technique. Their LB films exhibited optical second-harmonic generation (SHG). The chevron-shaped molecules have a central cationic acceptor and two pi-bridged donor groups with an angle of ca. 120 deg between the charge-transfer axes of the D-pi-(A sup +)-pi-D unit. A monolayer LB film of a representative example, 1-butyl-2,6-bis[2- (4-dibutylaminophenyl)vinyl]pyridinium iodide, has an effective susceptibility, chi sup ( sup 2 sup ) sub e sub f sub f , of 120 pm V sup - sup 1 at 1064 nm, a thickness of 1.16 nm and an area in contact with the substrate of 0.91 nm sup 2 molecule sup - sup 1. The second-harmonic intensity (1.6 x 10 sup - sup 4 versus quartz) is similar to those of the extensively studied conventional amphiphilic hemicyanines but as a result of non-centrosymmetric alignment, without the need for long ...

  3. Interference control of nonlinear excitation in a multi-atom cavity quantum electrodynamics system.

    Science.gov (United States)

    Yang, Guoqing; Tan, Zheng; Zou, Bichen; Zhu, Yifu

    2014-12-01

    We show that by manipulating quantum interference in a multi-atom cavity quantum electrodynamics (CQED) system, the nonlinear excitation of the cavity-atom polariton can be resonantly enhanced while the linear excitation is suppressed. Under the appropriate conditions, it is possible to selectively enhance or suppress the polariton excitation with two free-pace laser fields. We report on an experiment with cold Rb atoms in an optical cavity and present experimental results that demonstrate such interference control of the CQED excitation and its direct application to studies of all-optical switching and cross-phase modulation of the cavity-transmitted light.

  4. Chaos and Nonlinear Dynamics in a Quantum Artificial Economy

    CERN Document Server

    Gonçalves, Carlos Pedro

    2012-01-01

    Chaos and nonlinear economic dynamics are addressed for a quantum coupled map lattice model of an artificial economy, with quantized supply and demand equilibrium conditions. The measure theoretic properties and the patterns that emerge in both the economic business volume dynamics' diagrams as well as in the quantum mean field averages are addressed and conclusions are drawn in regards to the application of quantum chaos theory to address signatures of chaotic dynamics in relevant discrete economic state variables.

  5. Time-reversed wave mixing in nonlinear optics.

    Science.gov (United States)

    Zheng, Yuanlin; Ren, Huaijin; Wan, Wenjie; Chen, Xianfeng

    2013-11-19

    Time-reversal symmetry is important to optics. Optical processes can run in a forward or backward direction through time when such symmetry is preserved. In linear optics, a time-reversed process of laser emission can enable total absorption of coherent light fields inside an optical cavity of loss by time-reversing the original gain medium. Nonlinearity, however, can often destroy such symmetry in nonlinear optics, making it difficult to study time-reversal symmetry with nonlinear optical wave mixings. Here we demonstrate time-reversed wave mixings for optical second harmonic generation (SHG) and optical parametric amplification (OPA) by exploring this well-known but underappreciated symmetry in nonlinear optics. This allows us to observe the annihilation of coherent beams. Our study offers new avenues for flexible control in nonlinear optics and has potential applications in efficient wavelength conversion, all-optical computing.

  6. Quantum optical dipole radiation fields

    CERN Document Server

    Stokes, Adam

    2016-01-01

    We introduce quantum optical dipole radiation fields defined in terms of photon creation and annihilation operators. These fields are identified through their spatial dependence, as the components of the total fields that survive infinitely far from the dipole source. We use these radiation fields to perturbatively evaluate the electromagnetic radiated energy-flux of the excited dipole. Our results indicate that the standard interpretation of a bare atom surrounded by a localised virtual photon cloud, is difficult to sustain, because the radiated energy-flux surviving infinitely far from the source contains virtual contributions. It follows that there is a clear distinction to be made between a radiative photon defined in terms of the radiation fields, and a real photon, whose identification depends on whether or not a given process conserves the free energy. This free energy is represented by the difference between the total dipole-field Hamiltonian and its interaction component.

  7. Making of a nonlinear optical cavity

    CERN Document Server

    Martínez-Lorente, R; Esteban-Martín, A; García-Monreal, J; Roldán, E; Silva, F

    2016-01-01

    In the article we explain in detail how to build a photorefractive oscillator (PRO), which is a laser-pumped nonlinear optical cavity containing a photorefractive crystal. The specific PRO whose construction we describe systematically, is based on a Fabry-Perot optical cavity working in a non-degenerate four wave-mixing configuration. This particular PRO has the property that the generated beam exhibits laser-like phase invariance and, as an application, we show how a suitably modulated injected beam converts the output field from phase-invariant into phase-bistable. While the emphasis is made on the making of the experimental device and on the way measurements are implemented, some introduction to the photorefractive effect as well as to the necessary concepts of nonlinear dynamics are also given, so that the article is reasonably self-contained.

  8. Impact of nonlinearities on fiber optic communications

    CERN Document Server

    2011-01-01

    This book covers the recent progress in fiber-optic communication systems with a main focus on the impact of fiber nonlinearities on system performance. There has been significant progress in coherent communication systems in the past few years due to the advances in digital signal processing techniques. This has led to renewed interest in fiber linear and nonlinear impairments as well as techniques to mitigate them in the electrical domain. In this book, the reader will find all the important topics of fiber optic communication systems in one place, with in-depth coverage by the experts of each sub-topic. Pioneers from each of the sub-topics have been invited to contribute. Each chapter will have a section on fundamentals as well as reviews of literature and of recent developments. Readers will benefit from this approach since many of the conference proceedings and journal articles mainly focus on the authors’ research, without spending space on preliminaries.

  9. Nonlinear optics of astaxanthin thin films

    Science.gov (United States)

    Esser, A.; Fisch, Herbert; Haas, Karl-Heinz; Haedicke, E.; Paust, J.; Schrof, Wolfgang; Ticktin, Anton

    1993-02-01

    Carotinoids exhibit large nonlinear optical properties due to their extended (pi) -electron system. Compared to other polyenes which show a broad distribution of conjugation lengths, carotinoids exhibit a well defined molecular structure, i.e. a well defined conjugation length. Therefore the carotinoid molecules can serve as model compounds to study the relationship between structure and nonlinear optical properties. In this paper the synthesis of four astaxanthins with C-numbers ranging from 30 to 60, their preparation into thin films, wavelength dispersive Third Harmonic Generation (THG) measurements and some molecular modelling calculations will be presented. Resonant (chi) (3) values reach 1.2(DOT)10-10 esu for C60 astaxanthin. In the nonresonant regime a figure of merit (chi) (3)/(alpha) of several 10-13 esu-cm is demonstrated.

  10. Nonlinear optical studies of organic monolayers

    Energy Technology Data Exchange (ETDEWEB)

    Shen, Y.R.

    1988-02-01

    Second-order nonlinear optical effects are forbidden in a medium with inversion symmetry, but are necessarily allowed at a surface where the inversion summary is broken. They are often sufficiently strong so that a submonolayer perturbation of the surface can be readily detected. They can therefore be used as effective tools to study monolayers adsorbed at various interfaces. We discuss here a number of recent experiments in which optical second harmonic generation (SHG) and sum-frequency generation (SFG) are employed to probe and characterize organic monolayers. 15 refs., 5 figs.

  11. Scattering Induced Quantum Interference of Multiple Quantum Optical States

    DEFF Research Database (Denmark)

    Ott, Johan Raunkjær; Wubs, Martijn; Mortensen, N. Asger;

    2011-01-01

    Using a discrete mode theory for propagation of quantum optical states, we investigate the consequences of multiple scattering on the degree of quadrature entanglement and quantum interference. We report that entangled states can be created by multiple-scattering. We furthermore show that quantum...... interference induced by the transmission of quantized light through a multiple-scattering medium will persist even after averaging over an ensemble of scattering samples....

  12. Topological nature of nonlinear optical effects in solids

    OpenAIRE

    Morimoto, Takahiro; Nagaosa, Naoto

    2015-01-01

    There are a variety of nonlinear optical effects including higher harmonic generations, photovoltaic effects, and nonlinear Kerr rotations. They are realized by the strong light irradiation to materials that results in nonlinear polarizations in the electric field. These are of great importance in studying the physics of excited states of the system as well as for applications to optical devices and solar cells. Nonlinear properties of materials are usually described by the nonlinear suscepti...

  13. Enhanced optical nonlinearities in air-cladding silicon pedestal waveguides

    CERN Document Server

    Zhang, Yaojing; Yao, Yifei; Tsang, Hon Ki

    2016-01-01

    The third-order optical nonlinearity in optical waveguides has found applications in optical switching, optical wavelength conversion, optical frequency comb generation, and ultrafast optical signal processing. The development of an integrated waveguide platform with a high nonlinearity is therefore important for nonlinear integrated photonics. Here, we report the observation of an enhancement in the nonlinearity of an air-cladding silicon pedestal waveguide. We observe enhanced nonlinear spectral broadening compared to a conventional silicon-on-insulator waveguide. At the center wavelength of 1555 nm, the nonlinear-index coefficient of air-cladding silicon pedestal waveguide is measured to be about 5% larger than that of a conventional silicon-on-insulator waveguide. We observe enhanced spectral broadening from self-phase modulation of an optical pulse in the pedestal waveguide. The interaction of light with the confined acoustic phonons in the pedestal structure gives rise to a larger nonlinear-index coeffi...

  14. Nonlinear inversion schemes for fluorescence optical tomography.

    Science.gov (United States)

    Freiberger, Manuel; Egger, Herbert; Scharfetter, Hermann

    2010-11-01

    Fluorescence optical tomography is a non-invasive imaging modality that employs the absorption and re-emission of light by fluorescent dyes. The aim is to reconstruct the fluorophore distribution in a body from measurements of light intensities at the boundary. Due to the diffusive nature of light propagation in tissue, fluorescence tomography is a nonlinear and severely ill-posed problem, and some sort of regularization is required for a stable solution. In this paper we investigate reconstruction methods based on Tikhonov regularization with nonlinear penalty terms, namely total-variation regularization and a levelset-type method using a nonlinear parameterization of the unknown function. Moreover, we use the full threedimensional nonlinear forward model, which arises from the governing system of partial differential equations. We discuss the numerical realization of the regularization schemes by Newtontype iterations, present some details of the discretization by finite element methods, and outline the efficient implementation of sensitivity systems via adjoint methods. As we will demonstrate in numerical tests, the proposed nonlinear methods provide better reconstructions than standard methods based on linearized forward models and linear penalty terms. We will additionally illustrate, that the careful discretization of the methods derived on the continuous level allows to obtain reliable, mesh independent reconstruction algorithms.

  15. Coherent optical pulse sequencer for quantum applications.

    Science.gov (United States)

    Hosseini, Mahdi; Sparkes, Ben M; Hétet, Gabriel; Longdell, Jevon J; Lam, Ping Koy; Buchler, Ben C

    2009-09-10

    The bandwidth and versatility of optical devices have revolutionized information technology systems and communication networks. Precise and arbitrary control of an optical field that preserves optical coherence is an important requisite for many proposed photonic technologies. For quantum information applications, a device that allows storage and on-demand retrieval of arbitrary quantum states of light would form an ideal quantum optical memory. Recently, significant progress has been made in implementing atomic quantum memories using electromagnetically induced transparency, photon echo spectroscopy, off-resonance Raman spectroscopy and other atom-light interaction processes. Single-photon and bright-optical-field storage with quantum states have both been successfully demonstrated. Here we present a coherent optical memory based on photon echoes induced through controlled reversible inhomogeneous broadening. Our scheme allows storage of multiple pulses of light within a chosen frequency bandwidth, and stored pulses can be recalled in arbitrary order with any chosen delay between each recalled pulse. Furthermore, pulses can be time-compressed, time-stretched or split into multiple smaller pulses and recalled in several pieces at chosen times. Although our experimental results are so far limited to classical light pulses, our technique should enable the construction of an optical random-access memory for time-bin quantum information, and have potential applications in quantum information processing.

  16. Nonlinear dynamics and quantum entanglement in optomechanical systems.

    Science.gov (United States)

    Wang, Guanglei; Huang, Liang; Lai, Ying-Cheng; Grebogi, Celso

    2014-03-21

    To search for and exploit quantum manifestations of classical nonlinear dynamics is one of the most fundamental problems in physics. Using optomechanical systems as a paradigm, we address this problem from the perspective of quantum entanglement. We uncover strong fingerprints in the quantum entanglement of two common types of classical nonlinear dynamical behaviors: periodic oscillations and quasiperiodic motion. There is a transition from the former to the latter as an experimentally adjustable parameter is changed through a critical value. Accompanying this process, except for a small region about the critical value, the degree of quantum entanglement shows a trend of continuous increase. The time evolution of the entanglement measure, e.g., logarithmic negativity, exhibits a strong dependence on the nature of classical nonlinear dynamics, constituting its signature.

  17. Editorial . Quantum fluctuations and coherence in optical and atomic structures

    Science.gov (United States)

    Eschner, Jürgen; Gatti, Alessandra; Maître, Agnès; Morigi, Giovanna

    2003-03-01

    From simple interference fringes, over molecular wave packets, to nonlinear optical patterns - the fundamental interaction between light and matter leads to the formation of structures in many areas of atomic and optical physics. Sophisticated technology in experimental quantum optics, as well as modern computational tools available to theorists, have led to spectacular achievements in the investigation of quantum structures. This special issue is dedicated to recent developments in this area. It presents a selection of examples where quantum dynamics, fluctuations, and coherence generate structures in time or in space or where such structures are observed experimentally. The examples range from coherence phenomena in condensed matter, over atoms in optical structures, entanglement in light and matter, to quantum patterns in nonlinear optics and quantum imaging. The combination of such seemingly diverse subjects formed the basis of a successful European TMR network, "Quantum Structures" (visit http://cnqo.phys.strath.ac.uk/~gianluca/QSTRUCT/). This special issue partly re.ects the results and collaborations of the network, going however well beyond its scope by including contributions from a global community and from many related topics which were not addressed directly in the network. The aim of this issue is to present side by side these di.erent topics, all of which are loosely summarized under quantum structures, to highlight their common aspects, their di.erences, and the progress which resulted from the mutual exchange of results, methods, and knowledge. To guide the reader, we have organized the articles into subsections which follow a rough division into structures in material systems and structures in optical .elds. Nevertheless, in the following introduction we point out connections between the contributions which go beyond these usual criteria, thus highlighting the truly interdisciplinary nature of quantum structures. Much of the progress in atom optics

  18. All-optical sampling based on quantum-dot semiconductor optical amplifier

    Science.gov (United States)

    Wu, Chen; Wang, Yongjun; Wang, Lina

    2016-11-01

    In recent years, the all-optical signal processing system has become a hot research field of optical communication. This paper focused on the basic research of quantum-dot (QD) semiconductor optical amplifier (SOA) and studied its practical application to all-optical sampling. A multi-level dynamic physical model of QD-SOA is established, and its ultrafast dynamic characteristics are studied through theoretical and simulation research. For further study, an all-optical sampling scheme based on the nonlinear polarization rotation (NPR) effect of QD-SOA is also proposed. This paper analyzed the characteristics of optical switch window and investigated the influence of different control light pulses on switch performance. The presented optical sampling method has an important role in promoting the improvement of all-optical signal processing technology.

  19. Quantum Popov robust stability analysis of an optical cavity containing a saturated Kerr medium

    Science.gov (United States)

    Petersen, Ian R.

    2017-09-01

    This paper applies results of the robust stability of nonlinear quantum systems to a system consisting of an optical cavity containing a saturated Kerr medium. The system is characterised by a Hamiltonian operator that contains a non-quadratic term involving a quartic function of the annihilation and creation operators. A saturated version of the Kerr nonlinearity leads to a sector-bounded nonlinearity that enables a quantum small gain theorem to be applied to this system in order to analyse its stability. Also, a non-quadratic version of a quantum Popov stability criterion is presented and applied to analyse the stability of this system.

  20. Quantum Modelling of Electro-Optic Modulators

    CERN Document Server

    Capmany, Jose

    2011-01-01

    Many components that are employed in quantum information and communication systems are well known photonic devices encountered in standard optical fiber communication systems, such as optical beamsplitters, waveguide couplers and junctions, electro-optic modulators and optical fiber links. The use of these photonic devices is becoming increasingly important especially in the context of their possible integration either in a specifically designed system or in an already deployed end-to-end fiber link. Whereas the behavior of these devices is well known under the classical regime, in some cases their operation under quantum conditions is less well understood. This paper reviews the salient features of the quantum scattering theory describing both the operation of the electro-optic phase and amplitude modulators in discrete and continuous-mode formalisms. This subject is timely and of importance in light of the increasing utilization of these devices in a variety of systems, including quantum key distribution an...

  1. A reversible optical to microwave quantum interface

    CERN Document Server

    Barzanjeh, Sh; Milburn, G J; Tombesi, P; Vitali, D

    2011-01-01

    Quantum technology, like many mature classical technologies, will ultimately integrate distinct modules to achieve a function that transcends the capability of any one of them. We describe a reversible quantum interface between an optical and a microwave photon using a hybrid device based on the common interaction of microwave and optical fields with a nano-mechanical resonator in a superconducting circuit, which is one of the major challenges in the field. The scheme provides a path for generating a traveling microwave field strongly entangled with an optical mode, thus bridging the gap between quantum optical and solid state implementations of quantum information. This is an effective source of (bright) two-mode squeezing with an optical idler (signal) and a microwave signal (idler) and as such enables a continuous variable teleportation protocol.

  2. Two-mode optical state truncation and generation of maximally entangled states in pumped nonlinear couplers

    CERN Document Server

    Miranowicz, A; Miranowicz, Adam; Leonski, Wieslaw

    2006-01-01

    Schemes for optical-state truncation of two cavity modes are analysed. The systems, referred to as the nonlinear quantum scissors devices, comprise two coupled nonlinear oscillators (Kerr nonlinear coupler) with one or two of them pumped by external classical fields. It is shown that the quantum evolution of the pumped couplers can be closed in a two-qubit Hilbert space spanned by vacuum and single-photon states only. Thus, the pumped couplers can behave as a two-qubit system. Analysis of time evolution of the quantum entanglement shows that Bell states can be generated. A possible implementation of the couplers is suggested in a pumped double-ring cavity with resonantly enhanced Kerr nonlinearities in an electromagnetically-induced transparency scheme. The fragility of the generated states and their entanglement due to the standard dissipation and phase damping are discussed by numerically solving two types of master equations.

  3. Photoconductivity, photoluminescence and optical Kerr nonlinear effects in zinc oxide films containing chromium nanoclusters

    Energy Technology Data Exchange (ETDEWEB)

    Torres-Torres, C., E-mail: crstorres@yahoo.com.mx [Seccion de Estudios de Posgrado e Investigacion, ESIME-Z, Instituto Politecnico Nacional, Mexico, DF 07738 (Mexico); Garcia-Cruz, M.L. [Centro de Investigacion en Dispositivos Semiconductores, Benemerita Universidad Autonoma de Puebla, A. P. J-48, Puebla 72570, Mexico (Mexico); Castaneda, L., E-mail: luisca@sirio.ifuap.buap.mx [Instituto de Fisica, Benemerita Universidad Autonoma de Puebla, A. P. J-48, Puebla 72570, Mexico (Mexico); Rangel Rojo, R. [CICESE/Depto. de Optica, A. P. 360, Ensenada, BC 22860 (Mexico); Tamayo-Rivera, L. [Instituto de Fisica, Universidad Nacional Autonoma de Mexico, Mexico, DF 01000 (Mexico); Maldonado, A. [Depto. de Ing. Electrica, CINVESTAV IPN-SEES, A. P. 14740, Mexico DF 07000 (Mexico); Avendano-Alejo, M., E-mail: imax_aa@yahoo.com.mx [Centro de Ciencias Aplicadas y Desarrollo Tecnologico, Universidad Nacional Autonoma de Mexico, A. P. 70-186, 04510, DF (Mexico); and others

    2012-04-15

    Chromium doped zinc oxide thin solid films were deposited on soda-lime glass substrates. The photoconductivity of the material and its influence on the optical behavior was evaluated. A non-alkoxide sol-gel synthesis approach was used for the preparation of the samples. An enhancement of the photoluminescence response exhibited by the resulting photoconductive films with embedded chromium nanoclusters is presented. The modification in the photoconduction induced by a 445 nm wavelength was measured and then associated with the participation of the optical absorptive response. In order to investigate the third order optical nonlinearities of the samples, a standard time-resolved Optical Kerr Gate configuration with 80 fs pulses at 830 nm was used and a quasi-instantaneous pure electronic nonlinearity without the contribution of nonlinear optical absorption was observed. We estimate that from the inclusion of Cr nanoclusters into the sample results a strong optical Kerr effect originated by quantum confinement. The large photoluminescence response and the important refractive nonlinearity of the photoconductive samples seem to promise potential applications for the development of multifunctional all-optical nanodevices. - Highlights: Black-Right-Pointing-Pointer Enhancement in photoluminescence for chromium doped zinc oxide films is presented. Black-Right-Pointing-Pointer A strong and ultrafast optical Kerr effect seems to result from quantum confinement. Black-Right-Pointing-Pointer Photoconductive properties for optical and optoelectronic functions were observed.

  4. Quantum mechanics of charged particle beam optics

    CERN Document Server

    Khan, Sameen Ahmed

    2018-01-01

    Theory of charged particle beam optics is basic to the design and working of charged particle beam devices from electron microscopes to accelerator machines. Traditionally, the optical elements of the devices are designed and operated based on classical mechanics and classical electromagnetism, and only certain specific quantum mechanical aspects are dealt with separately using quantum theory. This book provides a systematic approach to quantum theory of charged particle beam optics, particularly in the high energy cases such as accelerators or high energy electron microscopy.

  5. Generalized optomechanics and its applications quantum optical properties of generalized optomechanical system

    CERN Document Server

    Li, Jin Jin

    2013-01-01

    A mechanical oscillator coupled to the optical field in a cavity is a typical cavity optomechanical system. In our textbook, we prepare to introduce the quantum optical properties of optomechanical system, i.e. linear and nonlinear effects. Some quantum optical devices based on optomechanical system are also presented in the monograph, such as the Kerr modulator, quantum optical transistor, optomechanical mass sensor, and so on. But most importantly, we extend the idea of typical optomechanical system to coupled mechanical resonator system and demonstrate that the combined two-level structure

  6. Optically active quantum-dot molecules.

    Science.gov (United States)

    Shlykov, Alexander I; Baimuratov, Anvar S; Baranov, Alexander V; Fedorov, Anatoly V; Rukhlenko, Ivan D

    2017-02-20

    Chiral molecules made of coupled achiral semiconductor nanocrystals, also known as quantum dots, show great promise for photonic applications owing to their prospective uses as configurable building blocks for optically active structures, materials, and devices. Here we present a simple model of optically active quantum-dot molecules, in which each of the quantum dots is assigned a dipole moment associated with the fundamental interband transition between the size-quantized states of its confined charge carriers. This model is used to analytically calculate the rotatory strengths of optical transitions occurring upon the excitation of chiral dimers, trimers, and tetramers of general configurations. The rotatory strengths of such quantum-dot molecules are found to exceed the typical rotatory strengths of chiral molecules by five to six orders of magnitude. We also study how the optical activity of quantum-dot molecules shows up in their circular dichroism spectra when the energy gap between the molecular states is much smaller than the states' lifetime, and maximize the strengths of the circular dichroism peaks by optimizing orientations of the quantum dots in the molecules. Our analytical results provide clear design guidelines for quantum-dot molecules and can prove useful in engineering optically active quantum-dot supercrystals and photonic devices.

  7. Third-Order Nonlinear Optical Susceptibility of Indium Phosphide Nanocrystals

    Institute of Scientific and Technical Information of China (English)

    WANG Hong-Li; WANG Dong; CHEN Guang-De; LIU Hui

    2007-01-01

    InP nanocrystals synthesized by refluxing and annealing of organic solvent are determined from XRD measurements to have an average granularity of 25 nm. The nonlinear optical properties of the InP nanocrystals studied by using laser Z-scan technique with 50ps pulses at 532nm are found to reveal strong nonlinear optical properties and two-photon absorption phenomenon. Also, the nonlinear absorption coefficient, the nonlinear refractive index and the third-order nonlinear optical susceptibility are determined by experiments, in which the nonlinear refractive index is three orders of magnitude larger than that of bulk InP.

  8. Quantum optical coherence in cytoskeletal microtubules: implications for brain function.

    Science.gov (United States)

    Jibu, M; Hagan, S; Hameroff, S R; Pribram, K H; Yasue, K

    1994-01-01

    'Laser-like,' long-range coherent quantum phenomena may occur biologically within cytoskeletal microtubules. This paper presents a theoretical prediction of the occurrence in biological media of the phenomena which we term 'superradiance' and 'self-induced transparency'. Interactions between the electric dipole field of water molecules confined within the hollow core of microtubules and the quantized electromagnetic radiation field are considered, and microtubules are theorized to play the roles of non-linear coherent optical devices. Superradiance is a specific quantum mechanical ordering phenomenon with characteristic times much shorter than those of thermal interaction. Consequently, optical signalling (and computation) in microtubules would be free from both thermal noise and loss. Superradiant optical computing in networks of microtubules and other cytoskeletal structures may provide a basis for biomolecular cognition and a substrate for consciousness.

  9. DSP Approach to the Design of Nonlinear Optical Devices

    Directory of Open Access Journals (Sweden)

    Steve Blair

    2005-06-01

    Full Text Available Discrete-time signal processing (DSP tools have been used to analyze numerous optical filter configurations in order to optimize their linear response. In this paper, we propose a DSP approach to design nonlinear optical devices by treating the desired nonlinear response in the weak perturbation limit as a discrete-time filter. Optimized discrete-time filters can be designed and then mapped onto a specific optical architecture to obtain the desired nonlinear response. This approach is systematic and intuitive for the design of nonlinear optical devices. We demonstrate this approach by designing autoregressive (AR and autoregressive moving average (ARMA lattice filters to obtain a nonlinear phase shift response.

  10. Optical dynamics in low-dimensional semiconductor heterostructures. Quantum dots and quantum cascade lasers

    Energy Technology Data Exchange (ETDEWEB)

    Weber, Carsten

    2008-07-01

    This work is focused on the optical dynamics of mesoscopic semiconductor heterostructures, using as prototypes zero-dimensional quantum dots and quantum cascade lasers which consist of quasitwo- dimensional quantum wells. Within a density matrix theory, a microscopic many-particle theory is applied to study scattering effects in these structures: the coupling to external as well as local fields, electron-phonon coupling, coupling to impurities, and Coulomb coupling. For both systems, the investigated effects are compared to experimentally observed results obtained during the past years. In quantum dots, the three-dimensional spatial confinement leads to the necessity to consider a quantum kinetic description of the dynamics, resulting in non-Markovian electron-phonon effects. This can be seen in the spectral phonon sidebands due to interaction with acoustic phonons as well as a damping of nonlinear Rabi oscillations which shows a nonmonotonous intensity and pulse duration dependence. An analysis of the inclusion of the self-interaction of the quantum dot shows that no dynamical local field terms appear for the simple two-level model. Considering local fields which have their origin in many quantum dots, consequences for a two-level quantum dot such as a zero-phonon line broadening and an increasing signal in photon echo experiments are found. For the use of quantum dots in an optical spin control scheme, it is found that the dephasing due to the electron-phonon interaction can be dominant in certain regimes. Furthermore, soliton and breather solutions are studied analytically in nonlinear quantum dot ensembles. Generalizing to quasi-two-dimensional structures, the intersubband dynamics of quantum cascade laser structures is investigated. A dynamical theory is considered in which the temporal evolution of the subband populations and the current density as well as the influence of scattering effects is studied. In the nonlinear regime, the scattering dependence and

  11. Quantum Sensors: Improved Optical Measurement via Specialized Quantum States

    Directory of Open Access Journals (Sweden)

    David S. Simon

    2016-01-01

    Full Text Available Classical measurement strategies in many areas are approaching their maximum resolution and sensitivity levels, but these levels often still fall far short of the ultimate limits allowed by the laws of physics. To go further, strategies must be adopted that take into account the quantum nature of the probe particles and that optimize their quantum states for the desired application. Here, we review some of these approaches, in which quantum entanglement, the orbital angular momentum of single photons, and quantum interferometry are used to produce optical measurements beyond the classical limit.

  12. UV Nano-Lights - Nonlinear Quantum Dot-Plasmon Coupling

    Science.gov (United States)

    2016-06-20

    nanomaterials systems for nonlinear optics. PROJECT TIMELINE The project timeline was segmented into 3 monthly intervals. The PhD students, assisted by...technique to remove the scattering component of light from the fluorescence emission with commonly-used fluorometers [Shortell, Optics Express...nanostructure light interaction and also has helped understand and remove unwanted signal contamination through optical element interference effects as

  13. Quantum optics and frontiers of physics: the third quantum revolution

    Science.gov (United States)

    Celi, Alessio; Sanpera, Anna; Ahufinger, Veronica; Lewenstein, Maciej

    2017-01-01

    The year 2015 was the International Year of Light. However, it also marked, the 20th anniversary of the first observation of Bose-Einstein condensation in atomic vapors by Eric Cornell, Carl Wieman and Wolfgang Ketterle. This discovery could be considered as one of the greatest achievements of quantum optics that has triggered an avalanche of further seminal discoveries and achievements. For this reason we devote this essay for the focus issue on ‘Quantum Optics in the International Year of Light’ to the recent revolutionary developments in quantum optics at the frontiers of all physics: atomic physics, molecular physics, condensed matter physics, high energy physics and quantum information science. We follow here the lines of the introduction to our book ‘Ultracold atoms in optical lattices: Simulating quantum many-body systems’ (Lewenstein et al 2012 Ultracold Atoms in Optical Lattices: Simulating Quantum Many-body Systems (Oxford: University Press)), and to a lesser extent the review article M Lewenstein et al (2007 Adv. Phys. 56 243). The book, however, was published in 2012, and many things has happened since then—the present essay is therefore upgraded to include the latest developments.

  14. Quantum cryptography over underground optical fibers

    Energy Technology Data Exchange (ETDEWEB)

    Hughes, R.J.; Luther, G.G.; Morgan, G.L.; Peterson, C.G.; Simmons, C.

    1996-05-01

    Quantum cryptography is an emerging technology in which two parties may simultaneously generated shared, secret cryptographic key material using the transmission of quantum states of light whose security is based on the inviolability of the laws of quantum mechanics. An adversary can neither successfully tap the key transmissions, nor evade detection, owing to Heisenberg`s uncertainty principle. In this paper the authors describe the theory of quantum cryptography, and the most recent results from their experimental system with which they are generating key material over 14-km of underground optical fiber. These results show that optical-fiber based quantum cryptography could allow secure, real-time key generation over ``open`` multi-km node-to-node optical fiber communications links between secure ``islands.``

  15. Atom-loss-induced quantum optical bi-stability switch

    Institute of Scientific and Technical Information of China (English)

    Wu Bao-Jun; Cui Fu-Cheng

    2012-01-01

    We investigate the nonlinear dynamics of a system composed of a cigar-shaped Bose-Einstein condensate and an optical cavity with the two sides coupled dispersively.By adopting discrete-mode approximation for the condensate,taking atom loss as a necessary part of the model to analyze the evolution of the system,while using trial and errormethod to find out steady states of the system as a reference,numerical simulation demonstrates that with a constant pump,atom loss will trigger a quantum optical bi-stability switch,which predicts a new interesting phenomenon for experiments to verify.

  16. Linear and nonlinear optical response of spherical anisotropic semiconductor microcrystallites

    Science.gov (United States)

    Ramaniah, Lavanya M.; Nair, Selvakumar V.; Rustagi, Kailash C.

    1989-12-01

    We present a phenomenological theory of the linear and nonlinear optical properties associated with the Fröhlich resonances of an optically anisotropic, spherical semiconductor crystallite. Using the Maxwell-Garnett approach, we calculate the effective dielectric function of a composite medium containing such crystallites. To study the effect of anisotropy, we take CdS and CdSe quantum dots as examples for the inclusions, and use a two-resonance model for the dielectric function. Even for randomly oriented inclusions, the Fröhlich resonances split as a result of anisotropic local-field corrections. At higher laser intensities, absorption saturation leads to bistability or tristability in the optical response of individual crystallites, while the response of the composite medium with randomly oriented inclusions shows multistability, with many intermediate branches. The nonlinear response of such a composite medium also exhibits a new kind of orientation-induced broadening of resonances. We also find that tristability is possible in another kind of inhomogeneous material, viz., a composite medium containing two types of isotropic spherical crystallites.

  17. Quantum optics in multiple scattering random media

    DEFF Research Database (Denmark)

    Lodahl, Peter

    Quantum Optics in Multiple Scattering Random Media Peter Lodahl Research Center COM, Technical University of Denmark, Dk-2800 Lyngby, Denmark. Coherent transport of light in a disordered random medium has attracted enormous attention both from a fundamental and application point of view. Coherent...... quantum optics in multiple scattering media and novel fundamental phenomena have been predicted when examining quantum fluctuations instead of merely the intensity of the light [1]. Here I will present the first experimental study of the propagation of quantum noise through an elastic, multiple scattering...... medium [2]. Two different types of quantum noise measurements have been carried out: total transmission and short-range frequency correlations. When comparing shot noise (quantum) to technical noise (classical) we observed markedly different behavior, c.f. Fig. 1. The experimental results are found...

  18. EDITORIAL The 17th Central European Workshop on Quantum Optics

    Science.gov (United States)

    Man'ko, Margarita A.

    2011-02-01

    -correlation function for graphs with and without time-reversal symmetry: the open system case Michał Ławniczak, Szymon Bauch, Oleh Hul and Leszek Sirko Independent nonclassical tests for states and measurements in the same experiment Alfredo Luis and Ángel Rivas On the classical capacity of quantum Gaussian channels Cosmo Lupo, Stefano Pirandola, Paolo Aniello and Stefano Mancini Entropic inequalities for center-of-mass tomograms Margarita A Man'ko Semiclassical dynamics for an ion confined within a nonlinear electromagnetic trap Bogdan M Mihalcea Zeno-like phenomena in STIRAP processes B Militello, M Scala, A Messina and N V Vitanov A beam splitter with second-order nonlinearity modeled as a nonlinear coupler V Peřinová, A Lukš and J Křepelka Energy-level shifts of a uniformly accelerated atom between two reflecting plates L Rizzuto and S Spagnolo Cross-Kerr nonlinearities in an optically dressed periodic medium K Słowik, A Raczyński, J Zaremba, S Zielińska-Kaniasty, M Artoni and G C La Rocca An approximate effective beamsplitter interaction between light and atomic ensembles Richard Tatham, David Menzies and Natalia Korolkova Stochastic simulation of long-time nonadiabatic dynamics Daniel A Uken, Alessandro Sergi and Francesco Petruccione

  19. Quantum stream cipher based on optical communications

    OpenAIRE

    Hirota, Osamu; Kato, Kentaro; Sohma, Masaki; Usuda, Tsuyoshi S.; HARASAWA, Katsuyoshi

    2004-01-01

    In 2000, an attractive new quantum cryptography was discovered by H.P.Yuen based on quantum communication theory. It is applicable to direct encryption, for example quantum stream cipher based on Yuen protocol(Y-00), with high speeds and for long distance by sophisticated optical devices which can work under the average photon number per signal light pulse:$ = 1000 \\sim 10000$. In addition, it may provide information-theoretic security against known/chosen plaintext attack, which has no class...

  20. Multiple Scattering of Quantum Optical States

    DEFF Research Database (Denmark)

    Ott, Johan Raunkjær; Mortensen, N. Asger; Lodahl, Peter

    2011-01-01

    fluctuations [3]. Only recently focus has reached the combination of quantum optics and multiple scattering, see e.g. references [4–7] and references therein. The experimental realization of strongly enhanced light-matter interaction in disordered photonic crystal waveguides, enabling cavity quantum...

  1. Optical Properties of Semiconductor Quantum Dots

    NARCIS (Netherlands)

    Perinetti, U.

    2011-01-01

    This thesis presents different optical experiments performed on semiconductor quantum dots. These structures allow to confine a small number of electrons and holes to a tiny region of space, some nm across. The aim of this work was to study the basic properties of different types of quantum dots

  2. Optical Properties of Semiconductor Quantum Dots

    NARCIS (Netherlands)

    Perinetti, U.

    2011-01-01

    This thesis presents different optical experiments performed on semiconductor quantum dots. These structures allow to confine a small number of electrons and holes to a tiny region of space, some nm across. The aim of this work was to study the basic properties of different types of quantum dots mad

  3. Progress in nonlinear nano-optics

    CERN Document Server

    Lienau, Christoph; Grunwald, Rüdiger

    2015-01-01

    This book presents the state of the art in nonlinear nanostructures for ultrafast laser applications. Most recent results in two emerging fields are presented: (i) generation of laser-induced nanostructures in materials like metals, metal oxides and semiconductors, and (ii) ultrafast excitation and energy transfer in nanoscale physical, chemical and hybrid systems. Particular emphasis is laid on the up-to-date controversially discussed mechanisms of sub-wavelength ripple formation including models of self-organized material transport and multiphoton excitation channels, nonlinear optics of plasmonic structures (nanotips, nanowires, 3D-metamaterials), and energy localization and transport on ultrafast time scale and spatial nanoscale. High-resolution spectroscopy, simulation and characterization techniques are reported. New applications of ultrashort-pulsed lasers for materials processing and the use of nanostructured materials for characterizing laser fields and laser-matter-interactions are discussed.

  4. Bacteriorhodopsin: Tunable Optical Nonlinear Magnetic Response

    CERN Document Server

    Bovino, F A; Sibilia, C; Giardina, M; Váró, G; Gergely, C

    2011-01-01

    We report on a strong and tunable magnetic optical nonlinear response of Bacteriorhodopsin (BR) under "off resonance" femtosecond (fs) pulse excitation, by detecting the polarization map of the noncollinear second harmonic signal of an oriented BR film, as a function of the input beam power. BR is a light-driven proton pump with a unique photochemistry initiated by the all trans retinal chromophore embedded in the protein. An elegant application of this photonic molecular machine has been recently found in the new area of optogenetics, where genetic expression of BR in brain cells conferred a light responsivity to the cells enabling thus specific stimulation of neurons. The observed strong tunable magnetic nonlinear response of BR might trigger promising applications in the emerging area of pairing optogenetics and functional magnetic resonance imaging susceptible to provide an unprecedented complete functional mapping of neural circuits.

  5. Universal quantum computation using all-optical hybrid encoding

    Institute of Scientific and Technical Information of China (English)

    郭奇; 程留永; 王洪福; 张寿

    2015-01-01

    By employing displacement operations, single-photon subtractions, and weak cross-Kerr nonlinearity, we propose an alternative way of implementing several universal quantum logical gates for all-optical hybrid qubits encoded in both single-photon polarization state and coherent state. Since these schemes can be straightforwardly implemented only using local operations without teleportation procedure, therefore, less physical resources and simpler operations are required than the existing schemes. With the help of displacement operations, a large phase shift of the coherent state can be obtained via currently available tiny cross-Kerr nonlinearity. Thus, all of these schemes are nearly deterministic and feasible under current technology conditions, which makes them suitable for large-scale quantum computing.

  6. Quantum Arnol'd Diffusion in a Simple Nonlinear System

    CERN Document Server

    Demikhovskii, V Y; Malyshev, A I

    2002-01-01

    We study the fingerprint of the Arnol'd diffusion in a quantum system of two coupled nonlinear oscillators with a two-frequency external force. In the classical description, this peculiar diffusion is due to the onset of a weak chaos in a narrow stochastic layer near the separatrix of the coupling resonance. We have found that global dependence of the quantum diffusion coefficient on model parameters mimics, to some extent, the classical data. However, the quantum diffusion happens to be slower that the classical one. Another result is the dynamical localization that leads to a saturation of the diffusion after some characteristic time. We show that this effect has the same nature as for the studied earlier dynamical localization in the presence of global chaos. The quantum Arnol'd diffusion represents a new type of quantum dynamics and can be observed, for example, in 2D semiconductor structures (quantum billiards) perturbed by time-periodic external fields.

  7. Nonlinear optical properties of induced transmission filters.

    Science.gov (United States)

    Owens, Daniel T; Fuentes-Hernandez, Canek; Hales, Joel M; Perry, Joseph W; Kippelen, Bernard

    2010-08-30

    The nonlinear optical (NLO) properties of induced transmission filters (ITFs) based on Ag are experimentally determined using white light continuum pump-probe measurements. The experimental results are supported using simulations based on the matrix transfer method. The magnitude of the NLO response is shown to be 30 times that of an isolated Ag film of comparable thickness. The impacts of design variations on the linear and NLO response are simulated. It is shown that the design can be modified to enhance the NLO response of an ITF by a factor of 2 or more over a perfectly matched ITF structure.

  8. Nonlinear Optics in AlGaAs on Insulator

    DEFF Research Database (Denmark)

    Pu, Minhao; Ottaviano, Luisa; Semenova, Elizaveta;

    2016-01-01

    AlGaAs on insulator is a powerful nonlinear platform sporting a high effective nonlinearity and the possibility to fabricate complex designs. We will present low loss waveguides enabling efficient optical signal processing and Kerr comb generation.......AlGaAs on insulator is a powerful nonlinear platform sporting a high effective nonlinearity and the possibility to fabricate complex designs. We will present low loss waveguides enabling efficient optical signal processing and Kerr comb generation....

  9. No-go theorem for passive single-rail linear optical quantum computing.

    Science.gov (United States)

    Wu, Lian-Ao; Walther, Philip; Lidar, Daniel A

    2013-01-01

    Photonic quantum systems are among the most promising architectures for quantum computers. It is well known that for dual-rail photons effective non-linearities and near-deterministic non-trivial two-qubit gates can be achieved via the measurement process and by introducing ancillary photons. While in principle this opens a legitimate path to scalable linear optical quantum computing, the technical requirements are still very challenging and thus other optical encodings are being actively investigated. One of the alternatives is to use single-rail encoded photons, where entangled states can be deterministically generated. Here we prove that even for such systems universal optical quantum computing using only passive optical elements such as beam splitters and phase shifters is not possible. This no-go theorem proves that photon bunching cannot be passively suppressed even when extra ancilla modes and arbitrary number of photons are used. Our result provides useful guidance for the design of optical quantum computers.

  10. Quantum-enhanced metrology with the single-mode coherent states of an optical cavity inside a quantum feedback loop

    Science.gov (United States)

    Clark, Lewis A.; Stokes, Adam; Beige, Almut

    2016-08-01

    In this paper, we use the nonlinear generator of dynamics of the individual quantum trajectories of an optical cavity inside an instantaneous quantum feedback loop to measure the phase shift between two pathways of light with a precision above the standard quantum limit. The feedback laser provides a reference frame and constantly increases the dependence of the state of the resonator on the unknown phase. Since our quantum metrology scheme can be implemented with current technology and does not require highly efficient single photon detectors, it should be of practical interest until highly entangled many-photon states become more readily available.

  11. Nonlinear interaction of electromagnetic field with quantum plasma

    CERN Document Server

    Latyshev, A V

    2014-01-01

    The analysis of nonlinear interaction of transversal electromagnetic field with quantum collisionless plasma is carried out. Formulas for calculation electric current in quantum collisionless plasma at any temperature are deduced. It has appeared, that the nonlinearity account leads to occurrence of the longitudinal electric current directed along a wave vector. This second current is orthogonal to the known transversal classical current, received at the classical linear analysis. The case of degenerate electronic plasma is considered. It is shown, that for degenerate plasmas the electric current is calculated under the formula, not containing quadratures.

  12. UV Nano Lights - Nonlinear Quantum Dot-Plasmon Coupling

    Science.gov (United States)

    2016-06-20

    AFRL-AFOSR-JP-TR-2016-0072 UV Nano-Lights - Nonlinear Quantum Dot-Plasmon Coupling Eric Waclawik QUEENSLAND UNIVERSITY OF TECHNOLOGY Final Report 06...Final 3.  DATES COVERED (From - To)  03 Feb 2014 to 02 Feb 2016 4.  TITLE AND SUBTITLE UV Nano-Lights - Nonlinear Quantum Dot-Plasmon Coupling 5a...CONTRACT NUMBER 5b.  GRANT NUMBER FA2386-14-1-4056 5c.   PROGRAM ELEMENT NUMBER 61102F 6.  AUTHOR(S) Eric Waclawik 5d.  PROJECT NUMBER 5e.  TASK NUMBER 5f

  13. Studies on the Second-Order Nonlinear Optical Properties of Parabolic and Semi-parabolic Quantum Wells with Applied Electric Fields

    Institute of Scientific and Technical Information of China (English)

    ZHANG Li; XIE Hong-Jing

    2004-01-01

    Within the framework of compact density matrix approach and iterative procedure, a detailed procedure for the calculation of the second-harmonic generation (SHG)susceptibility tensor is given in the electric-field-biased parabolic and semi-parabolic quantum wells (QWs). The simple analytical formula for the SHG susceptibility in the systems is also deduced. Numerical results on typical AlGaAs/GaAs materials show that, for the same effective width,the SHG susceptibility in semi-parabolic QW is larger than that in parabolic QW due to the self-asymmetry of the semiparabolic QW, and the applied electric field can make the SHG susceptibilities in both systems enhance remarkably.Moreover, the SHG susceptibility is also related to the parabolic confinement frequency and the relaxation rate of the systems.

  14. Nonlinear laser dynamics from quantum dots to cryptography

    CERN Document Server

    Lüdge, Kathy

    2012-01-01

    A distinctive discussion of the nonlinear dynamical phenomena of semiconductor lasers. The book combines recent results of quantum dot laser modeling with mathematical details and an analytic understanding of nonlinear phenomena in semiconductor lasers and points out possible applications of lasers in cryptography and chaos control. This interdisciplinary approach makes it a unique and powerful source of knowledge for anyone intending to contribute to this field of research.By presenting both experimental and theoretical results, the distinguished authors consider solitary lase

  15. Quantum dot devices for optical communications

    DEFF Research Database (Denmark)

    Mørk, Jesper

    2005-01-01

    . The main property of semiconductor quantum dots compared to bulk material or even quantum well structures is the discrete nature of the allowed states, which means that inversion of the medium can be obtained for very low electron densities. This has led to the fabrication of quantum dot lasers with record......-low threshold currents and amplifiers with record-high power levels. In this tutorial we will review the basic properties of quantum dots, emphasizing the properties which are important for laser and amplifier applications, as well as devices for all-optical signal processing. The high-speed properties...

  16. Enhancing a slow and weak optomechanical nonlinearity with delayed quantum feedback to implement a CPHASE gate

    CERN Document Server

    Wang, Zhaoyou

    2016-01-01

    We show that the effective optical nonlinearity of a cavity optomechanical system can be used to implement quantum gates between propagating photons. By using quantum feedback, we can enhance a slow and small optical nonlinearity to generate a large nonlinear phase shift between two spatially separated temporal modes of a propagating electromagnetic field. This allows us to implement a CPHASE gate between the two modes. After presenting a semiclassical derivation of the operation of the gate, we verify the result by a full simulation of the state of the quantum field in the waveguide coupled to a cavity. To efficiently solve the Schr\\"odinger equation of the full system, we develop a matrix product state approach that keeps track of the entangled full quantum state of the coupled system. These simulations verify the operation of the gate in the weak coupling regime where the semiclassical approximation is valid. In addition, we observe a major reduction in gate fidelity as we approach the vacuum strong coupli...

  17. Synthesis and quantum chemical studies of metalloorganics for electro-optical studies

    Science.gov (United States)

    Deepthi, S.; Jha, A.; Kumar, Ch. Ravi Shankar

    2017-07-01

    The dynamic nature of molecular materials are functional due to their nonlinear optical properties. Nonlinearity arising due to intermolecular interactions as self assembling phenomena between organic and metallic nanoparticles is of interest. The insight of this phenomena is attributed both by experimental and quantum chemical studies. Vibration studies performed by FTIR reveal intermolecular bonding forming metalloorganic POMZ with PAA and zinc oxide. These wave numbers were in agreement with theoretical studies performed by Gaussian 03v software package with B3LYP/6-31G basis set. Nonlinear optical properties such as energy difference, dipole moment, electronegativity, electrophylicity index and polarizability were attributed for electrical and optical properties of the material.

  18. High sensitivity optically pumped quantum magnetometer.

    Science.gov (United States)

    Tiporlini, Valentina; Alameh, Kamal

    2013-01-01

    Quantum magnetometers based on optical pumping can achieve sensitivity as high as what SQUID-based devices can attain. In this paper, we discuss the principle of operation and the optimal design of an optically pumped quantum magnetometer. The ultimate intrinsic sensitivity is calculated showing that optimal performance of the magnetometer is attained with an optical pump power of 20 μW and an operation temperature of 48°C. Results show that the ultimate intrinsic sensitivity of the quantum magnetometer that can be achieved is 327 fT/Hz(½) over a bandwidth of 26 Hz and that this sensitivity drops to 130 pT/Hz(½) in the presence of environmental noise. The quantum magnetometer is shown to be capable of detecting a sinusoidal magnetic field of amplitude as low as 15 pT oscillating at 25 Hz.

  19. Quantum corrections to nonlinear ion acoustic wave with Landau damping

    Energy Technology Data Exchange (ETDEWEB)

    Mukherjee, Abhik; Janaki, M. S. [Saha Institute of Nuclear Physics, Calcutta (India); Bose, Anirban [Serampore College, West Bengal (India)

    2014-07-15

    Quantum corrections to nonlinear ion acoustic wave with Landau damping have been computed using Wigner equation approach. The dynamical equation governing the time development of nonlinear ion acoustic wave with semiclassical quantum corrections is shown to have the form of higher KdV equation which has higher order nonlinear terms coming from quantum corrections, with the usual classical and quantum corrected Landau damping integral terms. The conservation of total number of ions is shown from the evolution equation. The decay rate of KdV solitary wave amplitude due to the presence of Landau damping terms has been calculated assuming the Landau damping parameter α{sub 1}=√(m{sub e}/m{sub i}) to be of the same order of the quantum parameter Q=ℏ{sup 2}/(24m{sup 2}c{sub s}{sup 2}L{sup 2}). The amplitude is shown to decay very slowly with time as determined by the quantum factor Q.

  20. Quantum correlations in optical angle-orbital angular momentum variables.

    Science.gov (United States)

    Leach, Jonathan; Jack, Barry; Romero, Jacqui; Jha, Anand K; Yao, Alison M; Franke-Arnold, Sonja; Ireland, David G; Boyd, Robert W; Barnett, Stephen M; Padgett, Miles J

    2010-08-06

    Entanglement of the properties of two separated particles constitutes a fundamental signature of quantum mechanics and is a key resource for quantum information science. We demonstrate strong Einstein, Podolsky, and Rosen correlations between the angular position and orbital angular momentum of two photons created by the nonlinear optical process of spontaneous parametric down-conversion. The discrete nature of orbital angular momentum and the continuous but periodic nature of angular position give rise to a special sort of entanglement between these two variables. The resulting correlations are found to be an order of magnitude stronger than those allowed by the uncertainty principle for independent (nonentangled) particles. Our results suggest that angular position and orbital angular momentum may find important applications in quantum information science.

  1. Progress Toward Single-Photon-Level Nonlinear Optics in Crystalline Microcavities

    Science.gov (United States)

    Kowligy, Abijith S.

    Over the last two decades, the emergence of quantum information science has uncovered many practical applications in areas such as communications, imaging, and sensing where harnessing quantum features of Nature provides tremendous benefits over existing methods exploiting classical physical phenomena. In this effort, one of the frontiers of research has been to identify and utilize quantum phenomena that are not susceptible to environmental and parasitic noise processes. Quantum photonics has been at the forefront of these studies because it allows room-temperature access to its inherently quantum-mechanical features, and allows leveraging the mature telecommunication industry. Accompanying the weak environmental influence, however, are also weak optical nonlinearities. Efficient nonlinear optical interactions are indispensible for many of the existing protocols for quantum optical computation and communication, e.g. high-fidelity entangling quantum logic gates rely on large nonlinear responses at the one- or few-photon-level. While this has been addressed to a great extent by interfacing photons with single quantum emitters and cold atomic gases, scalability has remained elusive. In this work, we identify the macroscopic second-order nonlinear polarization as a robust platform to address this challenge, and utilize the recent advances in the burgeoning field of optical microcavities to enhance this nonlinear response. In particular, we show theoretically that by using the quantum Zeno effect, low-noise, single-photon-level optical nonlinearities can be realized in lithium niobate whispering-gallery-mode microcavities, and present experimental progress toward this goal. Using the measured strength of the second-order nonlinear response in lithium niobate, we modeled the nonlinear system in the strong coupling regime using the Schrodinger picture framework and theoretically demonstrated that the single-photon-level operation can be observed for cavity lifetimes in

  2. Enhanced Kerr electro-optic nonlinearity through cascaded Pockels effects

    CERN Document Server

    Li, Guang-Zhen; Jiang, Hao-Wei; Chen, Xian-Feng

    2015-01-01

    We demonstrated a large enhancement of Kerr electro-optic nonlinearity through cascaded Pockels effects in a domain inversion ferroelectric crystal. We designed a structure that can implement the cascaded Pockels effects and second-harmonic generation simultaneously. The energy coupling between the fundamental lights of different polarizations led to a large nonlinear phase shift, and thus an effective electro-optic nonlinear refractive index. The effective nonlinearity can be either positive or negative, causing the second-harmonic spectra to move towards the coupling center, which in turn, offered us a way to measure the effective electro-optic nonlinear refractive index. The corresponding enhanced Kerr electro-optic nonlinearity is more than three orders of magnitude higher than the intrinsic value. These results open a door to manipulate the nonlinear phase by applying external electric field instead of light intensity in noncentrosymmetric crystals.

  3. Higher order nonlinearity and synchronization of quantum cascade lasers

    Institute of Scientific and Technical Information of China (English)

    Taraprasad Chattopadhyay; Prosenjit Bhattacharyya

    2011-01-01

    This paper presents a closed-form analysis of the synchronization phenomenon of the quantum cascade laser (QCL). The analysis has been made with considering higher order nonlinearity of the modal gain of the QCL. The frequency response characteristics of the synchronized QCL along with the stability of the locked state, the effect of nonlinearity on the lockband of the QCL and the amplitude limiting action of the locked QCL have been calculated. The analysis demonstrates the effect of higher order nonlinearity on the properties of the synchronized QCL.

  4. Quantum optics with quantum dots in photonic nanowires

    DEFF Research Database (Denmark)

    Claudon, Julien; Munsch, Matthieu; Bleuse, Joel;

    2012-01-01

    Besides microcavities and photonic crystals, photonic nanowires have recently emerged as a novel resource for solidstate quantum optics. We will review recent studies which demonstrate an excellent control over the spontaneous emission of InAs quantum dots (QDs) embedded in single-mode Ga...... quantum optoelectronic devices. Quite amazingly, this approach has for instance permitted (unlike microcavity-based approaches) to combine for the first time a record-high efficiency (72%) and a negligible g(2) in a QD single photon source....

  5. Evaluation of third order nonlinear optical parameters of CdS/PVA nanocomposite

    Energy Technology Data Exchange (ETDEWEB)

    Sharma, Mamta [Department of Physics, Center of Advanced Study in Physics, Panjab University, Chandigarh-160014 (India); Department of Applied Sciences (Physics), UIET, Panjab University, Chandigarh-160014 (India); Tripathi, S. K., E-mail: surya@pu.ac.in, E-mail: surya-tr@yahoo.com [Department of Physics, Center of Advanced Study in Physics, Panjab University, Chandigarh-160014 (India)

    2015-06-24

    CdS nanoparticles dispersed in PVA are prepared by Chemical method at room temperature. The nonlinear optical parameters such as nonlinear absorption (β), nonlinear refractive index (n{sub 2}) and nonlinear susceptibility (χ{sup 3}) are calculated for this sample by using Z-scan technique. CdS/PVA samples show the two photon absorption mechanism. The third order nonlinear susceptibility is calculated from n{sub 2} and β and is found to be of the order of 10{sup −7} – 10{sup −8} m{sup 2}/V{sup 2}. The larger value of third order nonlinear susceptibility is due to dielectric and quantum confinement effect.

  6. Quantum Computation Using Optically Coupled Quantum Dot Arrays

    Science.gov (United States)

    Pradhan, Prabhakar; Anantram, M. P.; Wang, K. L.; Roychowhury, V. P.; Saini, Subhash (Technical Monitor)

    1998-01-01

    A solid state model for quantum computation has potential advantages in terms of the ease of fabrication, characterization, and integration. The fundamental requirements for a quantum computer involve the realization of basic processing units (qubits), and a scheme for controlled switching and coupling among the qubits, which enables one to perform controlled operations on qubits. We propose a model for quantum computation based on optically coupled quantum dot arrays, which is computationally similar to the atomic model proposed by Cirac and Zoller. In this model, individual qubits are comprised of two coupled quantum dots, and an array of these basic units is placed in an optical cavity. Switching among the states of the individual units is done by controlled laser pulses via near field interaction using the NSOM technology. Controlled rotations involving two or more qubits are performed via common cavity mode photon. We have calculated critical times, including the spontaneous emission and switching times, and show that they are comparable to the best times projected for other proposed models of quantum computation. We have also shown the feasibility of accessing individual quantum dots using the NSOM technology by calculating the photon density at the tip, and estimating the power necessary to perform the basic controlled operations. We are currently in the process of estimating the decoherence times for this system; however, we have formulated initial arguments which seem to indicate that the decoherence times will be comparable, if not longer, than many other proposed models.

  7. Quantum optical signal processing in diamond

    CERN Document Server

    Fisher, Kent A G; Maclean, Jean-Phillipe W; Bustard, Philip J; Resch, Kevin J; Sussman, Benjamin J

    2015-01-01

    Controlling the properties of single photons is essential for a wide array of emerging optical quantum technologies spanning quantum sensing, quantum computing, and quantum communications. Essential components for these technologies include single photon sources, quantum memories, waveguides, and detectors. The ideal spectral operating parameters (wavelength and bandwidth) of these components are rarely similar; thus, frequency conversion and spectral control are key enabling steps for component hybridization. Here we perform signal processing of single photons by coherently manipulating their spectra via a modified quantum memory. We store 723.5 nm photons, with 4.1 nm bandwidth, in a room-temperature diamond crystal; upon retrieval we demonstrate centre frequency tunability over 4.2 times the input bandwidth, and bandwidth modulation between 0.5 to 1.9 times the input bandwidth. Our results demonstrate the potential for diamond, and Raman memories in general, to be an integrated platform for photon storage ...

  8. Third-order nonlinear optical response of Ag-CdSe/PVA hybrid nanocomposite

    Energy Technology Data Exchange (ETDEWEB)

    Tripathi, S.K.; Kaur, Ramneek; Kaur, Jaspreet; Sharma, Mamta [Panjab University, Department of Physics, Center of Advanced Study in Physics, Chandigarh (India)

    2015-09-15

    Hybrid nanocomposites of II-VI semiconductor nanoparticles are gaining great interest in nonlinear optoelectronic devices. Present work includes the characterization of CdSe polymer nanocomposite prepared by chemical in situ technique. From X-ray diffraction, the hexagonal wurtzite structure of nanoparticles has been confirmed with spherical morphology from transmission electron microscopy. Ag-CdSe hybrid polymer nanocomposite has been prepared chemically at different Ag concentrations. The presence of Ag in hybrid nanocomposite has been confirmed with energy-dispersive X-ray spectroscopy. The effect of varying Ag concentration on the linear and nonlinear optical properties of the nanocomposites has been studied. In linear optical parameters, the linear absorption coefficient, refractive index, extinction coefficient and optical conductivity have been calculated. The third-order nonlinear optical properties have been observed with open- and closed-aperture Z-scan technique. The large nonlinear refractive index ∝10{sup -5} cm{sup 2}/W with self-focusing behaviour is due to the combined effect of quantum confinement and thermo-optical effects. The enhanced nonlinearity with increasing Ag content is due to the surface plasmon resonance, which enhances the local electric field near the nanoparticle surface. Thus, Ag-CdSe hybrid polymer nanocomposite has favourable nonlinear optical properties for various optoelectronic applications. (orig.)

  9. Nonlinear quantum electrodynamic and electroweak processes in strong laser fields

    Energy Technology Data Exchange (ETDEWEB)

    Meuren, Sebastian

    2015-06-24

    Various nonlinear electrodynamic and electroweak processes in strong plane-wave laser fields are considered with an emphasis on short-pulse effects. In particular, the momentum distribution of photoproduced electron-positron pairs is calculated numerically and a semiclassical interpretation of its characteristic features is established. By proving the optical theorem, compact double-integral expressions for the total pair-creation probability are obtained and numerically evaluated. The exponential decay of the photon wave function in a plane wave is included by solving the Schwinger-Dyson equations to leading-order in the quasistatic approximation. In this respect, the polarization operator in a plane wave is investigated and its Ward-Takahashi identity verified. A classical analysis indicates that a photoproduced electron-positron pair recollides for certain initial conditions. The contributions of such recollision processes to the polarization operator are identified and calculated both analytically and numerically. Furthermore, the existence of nontrivial electron-spin dynamics induced by quantum fluctuations is verified for ultra-short laser pulses. Finally, the exchange of weak gauge bosons is considered, which is essential for neutrino-photon interactions. In particular, the axial-vector-vector coupling tensor is calculated and the so-called Adler-Bell-Jackiw (ABJ) anomaly investigated.

  10. Quantum Entanglement in Optical Lattice Systems

    Science.gov (United States)

    2015-02-18

    SECURITY CLASSIFICATION OF: Optical lattice systems provide an ideal platform for investigating entanglement because of their unprecedented level of...ABSTRACT Final report for ARO grant entitled "Quantum Entanglement in Optical Lattice Systems" Report Title Optical lattice systems provide an ideal ...2010): 0. doi: 10.1103/PhysRevA.82.063612 D. Blume, K. Daily. Breakdown of Universality for Unequal-Mass Fermi Gases with Infinite Scattering Length

  11. Highly nonlinear optical regime in graphene-assisted cavities: lasing threshold bares graphene nonlinearity

    CERN Document Server

    Ciattoni, Alessandro

    2014-01-01

    Strong nonlinear optical mechanisms operating in a miniaturized environment have a key role in photonics since they allow complex and versatile light manipulation within subwavelength devices. On the other hand, due to its two-dimensional planar geometry, graphene can easily be embedded within miniaturized structures and has fascinating linear and nonlinear optical properties arising from its relativistic electron dynamics. However, very few light steering graphene-based setups with a strong nonlinear behavior have been proposed since, due to its intrinsic planar localization, graphene nonlinearity has to be exploited through novel schemes not available in standard bulk nonlinear optics. Here we show that an active cavity hosting a graphene sheet, when tuned near its lasing threshold, is able to isolate the spatially localized graphene nonlinearity thus producing a very strong nonlinear device response with multi-valued features. The proposed strategy for exploiting graphene nonlinearity through its baring co...

  12. Electronic Structures of Asymmetrically Substituted Phthalocyanines and Their Second Non-linear Optical Properties

    Institute of Scientific and Technical Information of China (English)

    张天莉; 严继民

    2001-01-01

    Quantum-chemical AM1 calculations were performed to study the geometries,the electronic structures and the second nonlinear optical properties of phthalocyanine and some asymmetrically substituted phthalocyanines,which include tert-butyl,amino,dimethylamino,nitro,fluoro,chloro,bromo iodo and nitrile substituents. The relationships of the second nonlinear optical coefficients β with dipole moment μ, and β with the energy-gap differences of frontier orbitals ΔEDA were discussed. Two relationships are regular and all ΔEDA-μ show very good linear relationship.

  13. Nonlinear quantum mechanics, the superposition principle, and the quantum measurement problem

    Indian Academy of Sciences (India)

    Kinjalk Lochan; T P Singh

    2011-01-01

    There are four reasons why our present knowledge and understanding of quantum mechanics can be regarded as incomplete. (1) The principle of linear superposition has not been experimentally tested for position eigenstates of objects having more than about a thousand atoms. (2) There is no universally agreed upon explanation for the process of quantum measurement. (3) There is no universally agreed upon explanation for the observed fact that macroscopic objects are not found in superposition of position eigenstates. (4) Most importantly, the concept of time is classical and hence external to quantum mechanics: there should exist an equivalent reformulation of the theory which does not refer to an external classical time. In this paper we argue that such a reformulation is the limiting case of a nonlinear quantum theory, with the nonlinearity becoming important at the Planck mass scale. Such a nonlinearity can provide insights into the aforesaid problems. We use a physically motivated model for a nonlinear Schr ¨odinger equation to show that nonlinearity can help in understanding quantum measurement. We also show that while the principle of linear superposition holds to a very high accuracy for atomic systems, the lifetime of a quantum superposition becomes progressively smaller, as one goes from microscopic to macroscopic objects. This can explain the observed absence of position superpositions in macroscopic objects (lifetime is too small). It also suggests that ongoing laboratory experiments may be able to detect the finite superposition lifetime for mesoscopic objects in the near future.

  14. Integrated optic devices based on nonlinear optical polymers

    Science.gov (United States)

    van Tomme, Emmanuel; van Daele, Peter P.; Baets, Roel G.; Lagasse, Paul E.

    1991-03-01

    An examination is made of the state of the art of nonlinear optical polymeric materials in view of their potential advantages. It is shown that these organic materials have many attractive features compared to LiNbO3 and III-V semiconductors with regard to their use in integrated optic circuits, especially since the level of integration is ever increasing. Considering more specifically electro-optic devices, a description is given of some of the theoretical background and basic properties. These polymers have already demonstrated a very high and extremely fast electro-optic effect compared to LiNbO3. It is also shown how low-loss waveguides can be fabricated by using easy techniques such as direct UV bleaching. The performance of phase modulators, Mach-Zehnder interferometers, and 2 x 2 space switches built with such polymers is already very promising. The results described in this study indicate a rapid rate of progress made by this technology, and one can expect that polymers in general and NLO polymers in particular will play an increasingly important role in integrated optics.

  15. An exactly solvable three-dimensional nonlinear quantum oscillator

    Energy Technology Data Exchange (ETDEWEB)

    Schulze-Halberg, A. [Department of Mathematics and Actuarial Science, Indiana University Northwest, 3400 Broadway, Gary, Indiana 46408 (United States); Morris, J. R. [Department of Physics, Indiana University Northwest, 3400 Broadway, Gary, Indiana 46408 (United States)

    2013-11-15

    Exact analytical, closed-form solutions, expressed in terms of special functions, are presented for the case of a three-dimensional nonlinear quantum oscillator with a position dependent mass. This system is the generalization of the corresponding one-dimensional system, which has been the focus of recent attention. In contrast to other approaches, we are able to obtain solutions in terms of special functions, without a reliance upon a Rodrigues-type of formula. The wave functions of the quantum oscillator have the familiar spherical harmonic solutions for the angular part. For the s-states of the system, the radial equation accepts solutions that have been recently found for the one-dimensional nonlinear quantum oscillator, given in terms of associated Legendre functions, along with a constant shift in the energy eigenvalues. Radial solutions are obtained for all angular momentum states, along with the complete energy spectrum of the bound states.

  16. Nonlinearly-enhanced energy transport in many dimensional quantum chaos

    KAUST Repository

    Brambila, D. S.

    2013-08-05

    By employing a nonlinear quantum kicked rotor model, we investigate the transport of energy in multidimensional quantum chaos. This problem has profound implications in many fields of science ranging from Anderson localization to time reversal of classical and quantum waves. We begin our analysis with a series of parallel numerical simulations, whose results show an unexpected and anomalous behavior. We tackle the problem by a fully analytical approach characterized by Lie groups and solitons theory, demonstrating the existence of a universal, nonlinearly-enhanced diffusion of the energy in the system, which is entirely sustained by soliton waves. Numerical simulations, performed with different models, show a perfect agreement with universal predictions. A realistic experiment is discussed in two dimensional dipolar Bose-Einstein-Condensates (BEC). Besides the obvious implications at the fundamental level, our results show that solitons can form the building block for the realization of new systems for the enhanced transport of matter.

  17. Large nonlocal nonlinear optical response of castor oil

    Science.gov (United States)

    Souza, Rogério F.; Alencar, Márcio A. R. C.; Meneghetti, Mario R.; Hickmann, Jandir M.

    2009-09-01

    The nonlocal nonlinearity of castor oil was investigated using the Z-scan technique in the CW regime at 514 nm and in femtosecond regime at 810 nm. Large negative nonlinear refractive indexes of thermal origin, thermo-optical coefficients and degree of nonlocality were obtained for both laser excitation wavelengths. The results indicate that the electronic part of the nonlinear refractive index and nonlinear absorption were negligible. Our results suggest that castor oil is promising candidate as a nonlinear medium for several nonlocal optical applications, such as in spatial soliton propagation, as well as a dispersant agent in the measurement of absorptive properties of nanoparticles.

  18. Optical bistability in nonlinear composites with coated ellipsoidal nanoparticles

    CERN Document Server

    Pinchuk, A

    2003-01-01

    Nonlinear composite structures show great promise for use in optical switching, signal processing, etc. We derive an effective nonlinear dielectric permittivity of composite structures where coated ellipsoidal nonlinear particles are imbedded in a linear host medium. The derived expression for the effective dielectric permittivity tensor follows the Clasius-Mossotti approximation. We observe conditions for the existence of the optical bistability effect in a coated ellipsoidal particle with a nonlinear core and a metallic shell. Our numerical results show stronger bistability effects in more dense suspensions of nonlinear heterogeneous ellipsoids.

  19. Composite structures for the enhancement of nonlinear optical materials.

    Science.gov (United States)

    Neeves, A E; Birnboim, M H

    1988-12-01

    Calculations of the nonlinear optical behavior are developed for model composites consisting of nanospheres with a metallic core and a nonlinear shell suspended in a nonlinear medium. The concept for the enhancement of optical phase conjugation from all these nonlinear regions is that the optical field can be concentrated both inside and in the neighborhood of the metallic core, aided by surface-mediated plasmon resonance. Calculations for gold cores and aluminum cores indicate that phase-conjugate reflectivity enhancements of 10(8) may be possible.

  20. Quantum metrology. Optically measuring force near the standard quantum limit.

    Science.gov (United States)

    Schreppler, Sydney; Spethmann, Nicolas; Brahms, Nathan; Botter, Thierry; Barrios, Maryrose; Stamper-Kurn, Dan M

    2014-06-27

    The Heisenberg uncertainty principle sets a lower bound on the noise in a force measurement based on continuously detecting a mechanical oscillator's position. This bound, the standard quantum limit, can be reached when the oscillator subjected to the force is unperturbed by its environment and when measurement imprecision from photon shot noise is balanced against disturbance from measurement back-action. We applied an external force to the center-of-mass motion of an ultracold atom cloud in a high-finesse optical cavity and measured the resulting motion optically. When the driving force is resonant with the cloud's oscillation frequency, we achieve a sensitivity that is a factor of 4 above the standard quantum limit and consistent with theoretical predictions given the atoms' residual thermal disturbance and the photodetection quantum efficiency.

  1. Resonant Optical Absorption in Semiconductor Quantum Wells

    Institute of Scientific and Technical Information of China (English)

    YU Li-Yuan; CAO Jun-Cheng

    2004-01-01

    @@ We have calculated the intraband photon absorption coefficients of hot two-dimensional electrons interacting with polar-optical phonon modes in quantum wells. The dependence of the photon absorption coefficients on the photon wavelength λ is obtained both by using the quantum mechanical theory and by the balance-equation theory. It is found that the photon absorption spectrum displays a local resonant maximum, corresponding to LO energy, and the absorption peak vanishes with increasing the electronic temperature.

  2. Quantum Phases of Matter in Optical Lattices

    Science.gov (United States)

    2015-06-30

    findings contained in this report are those of the author(s) and should not contrued as an official Department of the Army position , policy or...phases in beyond-standard optical lattices”, Oct 25, 2013 Nikhil Monga, John Shumway, Kaden Hazzard, Erich Mueller, Steven Desch, " Renormalization of...Ho, “Cold Atoms in Curved Space ”, Quantum Materials-Perspectives and Opportunities, The Rice Center for Quantum Materials, December 15, 2014

  3. Characterizaticr of Solid State Laser and Nonlinear Optical Materials.

    Science.gov (United States)

    1995-02-02

    materials useful in the different methods for obtaining frequency agility: narrow line emitters with multiple lasing channels and nonlinear optical materials . In...codoped with two or more rare earth ions were studied and computers models developed to explain their spectral dynamics. The nonlinear optical materials investigated

  4. A Photonic Basis for Deriving Nonlinear Optical Response

    Science.gov (United States)

    Andrews, David L.; Bradshaw, David S.

    2009-01-01

    Nonlinear optics is generally first presented as an extension of conventional optics. Typically the subject is introduced with reference to a classical oscillatory electric polarization, accommodating correction terms that become significant at high intensities. The material parameters that quantify the extent of the nonlinear response are cast as…

  5. Nonlinear refractive index of optical crystals

    Science.gov (United States)

    Adair, Robert; Chase, L. L.; Payne, Stephen A.

    1989-02-01

    The nonlinear refractive indices (n2) of a large number of optical crystals have been measured at a wavelength near one micrometer with use of nearly degenerate three-wave mixing. The measurements are compared with the predictions of an empirical formula derived by Boling, Glass, and Owyoung. This formula, which relates n2 to the linear refractive index and its dispersion, is shown to be accurate to within about 30% for materials with nonlinear indices ranging over 3 orders of magnitude. Measurements for a number of binary oxide and fluoride crystals have been analyzed under the assumption that the hyperpolarizability of the anion is much larger than that of the cation. It is found that the hyperpolarizability of oxygen varies by a factor of 10, and that of fluorine varies by a factor of 7, depending on the size of the coordinating cation. This behavior is similar to that of the linear polarizability, although the hyperpolarizability is much more sensitive than the linear polarizability to the identity of the cation. The measured halide ion hyperpolarizabilities for several alkali-halide crystals are in reasonable agreement with recent self-consistent calculations. A semiempirical model was proposed by Wilson and Curtis to account for the dependence of the linear anionic polarizability on the radius of the cation. This model also accounts quite well for the variation of the hyperpolarizability of both fluorine and oxygen, except for cation partners that have filled or unfilled d-electron shells. The nonlinear indices of a number of complex oxides (i.e., those with more than one cation) have been calculated from the partial hyperpolarizabilities deduced from the data for the binary oxides. The calculated and measured values of n2 agree to within an average error of 13%.

  6. High nonlinear optical anisotropy of urea nanofibers

    Science.gov (United States)

    Isakov, D.; de Matos Gomes, E.; Belsley, M.; Almeida, B.; Martins, A.; Neves, N.; Reis, R.

    2010-07-01

    Nanofibers consisting of the optically nonlinear organic molecule urea embedded in both poly(ethylene oxide) (PEO) and poly(vinyl alcohol) (PVA) polymers were produced by the electrospinning technique. The second-harmonic generation produced by aligned fiber mats of these materials displays a strong dependence on the polarization of the incident light. In PVA-urea nanofibers the effectiveness in generating of the second-harmonic light is as high as that of a pure urea powder with an average grain size of 110 μm. The results suggest that single crystalline urea nanofibers were achieved with a long-range crystalline order extending into the range of 2-4 μm with PVA as the host polymer.

  7. Enhanced quantum communication via optical refocusing

    Energy Technology Data Exchange (ETDEWEB)

    Lupo, Cosmo [School of Science and Technology, University of Camerino, I-62032 Camerino (Italy); Giovannetti, Vittorio [National Enterprise for Nanoscience and Nanotechnology (NEST), Scuola Normale Superiore and Istituto Nanoscienze, Consiglio Nazionale delle Ricerche (CNR), I-56126 Pisa (Italy); Pirandola, Stefano [Department of Computer Science, University of York, York YO10 5GH (United Kingdom); Mancini, Stefano [School of Science and Technology, University of Camerino, I-62032 Camerino (Italy); Istituto Nazionale di Fisica Nucleare (INFN), Sezione di Perugia, I-06123 Perugia (Italy); Lloyd, Seth [Department of Mechanical Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States)

    2011-07-15

    We consider the problem of quantum communication mediated by a passive optical refocusing system. The model captures the basic features of all those situations in which a signal is either refocused by a repeater for long-distance communication, or it is focused on a detector prior to the information decoding process. Introducing a general method for linear passive optical systems, we determine the conditions under which optical refocusing implies information transmission gain. Although the finite aperture of the repeater may cause loss of information, we show that the presence of the refocusing system can substantially enhance the rate of reliable communication with respect to the free-space propagation. We explicitly address the transferring of classical messages over the quantum channel, but the results can be easily extended to include the case of transferring quantum messages as well.

  8. Enhanced quantum communication via optical refocusing

    Science.gov (United States)

    Lupo, Cosmo; Giovannetti, Vittorio; Pirandola, Stefano; Mancini, Stefano; Lloyd, Seth

    2011-07-01

    We consider the problem of quantum communication mediated by a passive optical refocusing system. The model captures the basic features of all those situations in which a signal is either refocused by a repeater for long-distance communication, or it is focused on a detector prior to the information decoding process. Introducing a general method for linear passive optical systems, we determine the conditions under which optical refocusing implies information transmission gain. Although the finite aperture of the repeater may cause loss of information, we show that the presence of the refocusing system can substantially enhance the rate of reliable communication with respect to the free-space propagation. We explicitly address the transferring of classical messages over the quantum channel, but the results can be easily extended to include the case of transferring quantum messages as well.

  9. Quantum vacuum radiation in optical glass

    CERN Document Server

    Liberati, Stefano; Visser, Matt

    2011-01-01

    A recent experimental claim of the detection of analogue Hawking radiation in an optical system [PRL 105 (2010) 203901] has led to some controversy [PRL 107 (2011) 149401, 149402]. While this experiment strongly suggests some form of particle creation from the quantum vacuum (and hence it is per se very interesting), it is also true that it seems difficult to completely explain all features of the observations by adopting the perspective of a Hawking-like mechanism for the radiation. For instance, the observed photons are emitted parallel to the optical horizon, and the relevant optical horizon is itself defined in an unusual manner by combining group and phase velocities. This raises the question: Is this really Hawking radiation, or some other form of quantum vacuum radiation? Naive estimates of the amount of quantum vacuum radiation generated due to the rapidly changing refractive index --- sometimes called the dynamical Casimir effect --- are not encouraging. However we feel that naive estimates could be ...

  10. Optical bistability in a nonlinear-shell-coated metallic nanoparticle

    Science.gov (United States)

    Chen, Hongli; Zhang, Youming; Zhang, Baile; Gao, Lei

    2016-01-01

    We provide a self-consistent mean field approximation in the framework of Mie scattering theory to study the optical bistability of a metallic nanoparticle coated with a nonlinear shell. We demonstrate that the nanoparticle coated with a weakly nonlinear shell exhibits optical bistability in a broad range of incident optical intensity. This optical bistability critically relies on the geometry of the shell-coated nanoparticle, especially the fractional volume of the metallic core. The incident wavelength can also affect the optical bistability. Through an optimization-like process, we find a design with broader bistable region and lower threshold field by adjusting the size of the nonlinear shell, the fractional volume of the metallic core, and the incident wavelength. These results may find potential applications in optical bistable devices such as all-optical switches, optical transistors and optical memories. PMID:26907967

  11. Quantum dot devices for optical communications

    DEFF Research Database (Denmark)

    Mørk, Jesper

    2005-01-01

    Semiconductor quantum dots are often described as "artificial atoms": They are small nanometre-sized structures in which electrons only are allowed to exist at certain discrete levels due to size quantization, thus allowing the engineering of fundamental properties such as the coupling to light....... The main property of semiconductor quantum dots compared to bulk material or even quantum well structures is the discrete nature of the allowed states, which means that inversion of the medium can be obtained for very low electron densities. This has led to the fabrication of quantum dot lasers with record......-low threshold currents and amplifiers with record-high power levels. In this tutorial we will review the basic properties of quantum dots, emphasizing the properties which are important for laser and amplifier applications, as well as devices for all-optical signal processing. The high-speed properties...

  12. Quantum Communication Experiments Over Optical Fiber

    Science.gov (United States)

    Takesue, Hiroki

    Quantum key distribution (QKD) is expected to be the first application of quantum information to be realized as a practical system. In the last decade, research on QKD made significant progress both in concept and technology. In this chapter, we review the progress of technologies designed to realize high-speed and long-distance quantum communication over optical fiber, focusing on the results obtained by NTT. The first section describes a roadmap towards scalable quantum communications, which is composed of three phases. The second section reviews our effort to realize phase 1 quantum communication systems, namely point-to-point QKD systems based on the differential phase shift QKD (DPS-QKD) protocol. The third section describes entanglement generation and application in the telecom band, which are the key technologies for realizing phase 2 and 3 systems. The final section provides a summary and describes the future outlook.

  13. Laser And Nonlinear Optical Materials For Laser Remote Sensing

    Science.gov (United States)

    Barnes, Norman P.

    2005-01-01

    NASA remote sensing missions involving laser systems and their economic impact are outlined. Potential remote sensing missions include: green house gasses, tropospheric winds, ozone, water vapor, and ice cap thickness. Systems to perform these measurements use lanthanide series lasers and nonlinear devices including second harmonic generators and parametric oscillators. Demands these missions place on the laser and nonlinear optical materials are discussed from a materials point of view. Methods of designing new laser and nonlinear optical materials to meet these demands are presented.

  14. Synchronous Optical Pumping of Quantum Revival Beats for Atomic Magnetometery

    CERN Document Server

    Seltzer, S J; Romalis, M V

    2006-01-01

    We observe quantum beats with periodic revivals due to non-linear spacing of Zeeman levels in the ground state of potassium atoms and demonstrate their synchronous optical pumping by double modulation of the pumping light at the Larmor frequency and the revival frequency. We show that synchronous pumping increases the degree of spin polarization by a factor of 4. As a practical example, we explore the application of this double-modulation technique to atomic magnetometers operating in the geomagnetic field range and find that it can increase the sensitivity and reduce magnetic field orientation-dependent measurement errors endemic to alkali-metal magnetometers.

  15. Quantum optics of lossy asymmetric beam splitters

    Science.gov (United States)

    Uppu, Ravitej; Wolterink, Tom A. W.; Tentrup, Tristan B. H.; Pinkse, Pepijn W. H.

    2016-07-01

    We theoretically investigate quantum interference of two single photons at a lossy asymmetric beam splitter, the most general passive 2$\\times$2 optical circuit. The losses in the circuit result in a non-unitary scattering matrix with a non-trivial set of constraints on the elements of the scattering matrix. Our analysis using the noise operator formalism shows that the loss allows tunability of quantum interference to an extent not possible with a lossless beam splitter. Our theoretical studies support the experimental demonstrations of programmable quantum interference in highly multimodal systems such as opaque scattering media and multimode fibers.

  16. Quantum optics of lossy asymmetric beam splitters

    CERN Document Server

    Uppu, Ravitej; Tentrup, Tristan B H; Pinkse, Pepijn W H

    2016-01-01

    We theoretically investigate quantum interference of two single photons at a lossy asymmetric beam splitter, the most general passive 2$\\times$2 optical circuit. The losses in the circuit result in a non-unitary scattering matrix with a non-trivial set of constraints on the elements of the scattering matrix. Our analysis using the noise operator formalism shows that the loss allows tunability of quantum interference to an extent not possible with a lossless beam splitter. Our theoretical studies support the experimental demonstrations of programmable quantum interference in highly multimodal systems such as opaque scattering media and multimode fibers.

  17. Quantum optical effective-medium theory and transformation quantum optics for metamaterials

    DEFF Research Database (Denmark)

    Wubs, Martijn; Amooghorban, Ehsan; Zhang, Jingjing

    2016-01-01

    While typically designed to manipulate classical light, metamaterials have many potential applications for quantum optics as well. We argue why a quantum optical effective-medium theory is needed. We present such a theory for layered metamaterials that is valid for light propagation in all spatial...... directions, thereby generalizing earlier work for one-dimensional propagation. In contrast to classical effective-medium theory there is an additional effective parameter that describes quantum noise. Our results for metamaterials are based on a rather general Lagrangian theory for the quantum...

  18. Quantum theory of nonlocal nonlinear Schrodinger equation

    CERN Document Server

    Vyas, Vivek M

    2015-01-01

    Nonlocal nonlinear Schrodinger model is quantised and exactly solved using the canonical framework. It is found that the usual canonical quantisation of the model leads to a theory with pathological inner product. This problem is resolved by constructing another inner product over the vector space of the theory. The resultant theory is found to be identical to that of nonrelativistic bosons with delta function interaction potential, devoid of any nonlocality. The exact eigenstates are found using the Bethe ansatz technique.

  19. Bidirectional all-optical switches based on highly nonlinear optical fibers

    Science.gov (United States)

    Liu, Wenjun; Yang, Chunyu; Liu, Mengli; Yu, Weitian; Zhang, Yujia; Lei, Ming; Wei, Zhiyi

    2017-05-01

    All-optical switches have become one of the research focuses of nonlinear optics due to their fast switching speed. They have been applied in such fields as ultrafast optics, all-optical communication and all-optical networks. In this paper, based on symbolic computation, bidirectional all-optical switches are presented using analytic two-soliton solutions. Various types of soliton interactions are analyzed through choosing the different parameters of high-order dispersion and nonlinearity. Results indicate that bidirectional all-optical switches can be effectively achieved using highly nonlinear optical fibers.

  20. Quantum Private Comparison Protocol with Linear Optics

    Science.gov (United States)

    Luo, Qing-bin; Yang, Guo-wu; She, Kun; Li, Xiaoyu

    2016-12-01

    In this paper, we propose an innovative quantum private comparison(QPC) protocol based on partial Bell-state measurement from the view of linear optics, which enabling two parties to compare the equality of their private information with the help of a semi-honest third party. Partial Bell-state measurement has been realized by using only linear optical elements in experimental measurement-device-independent quantum key distribution(MDI-QKD) schemes, which makes us believe that our protocol can be realized in the near future. The security analysis shows that the participants will not leak their private information.

  1. Resource-efficient linear optical quantum computation.

    Science.gov (United States)

    Browne, Daniel E; Rudolph, Terry

    2005-07-01

    We introduce a scheme for linear optics quantum computation, that makes no use of teleported gates, and requires stable interferometry over only the coherence length of the photons. We achieve a much greater degree of efficiency and a simpler implementation than previous proposals. We follow the "cluster state" measurement based quantum computational approach, and show how cluster states may be efficiently generated from pairs of maximally polarization entangled photons using linear optical elements. We demonstrate the universality and usefulness of generic parity measurements, as well as introducing the use of redundant encoding of qubits to enable utilization of destructive measurements--both features of use in a more general context.

  2. Optical limiter based on two-dimensional nonlinear photonic crystals

    Science.gov (United States)

    Belabbas, Amirouche; Lazoul, Mohamed

    2016-04-01

    The aim behind this work is to investigate the capabilities of nonlinear photonic crystals to achieve ultra-fast optical limiters based on third order nonlinear effects. The purpose is to combine the actions of nonlinear effects with the properties of photonic crystals in order to activate the photonic band according to the magnitude of the nonlinear effects, themselves a function of incident laser power. We are interested in designing an optical limiter based nonlinear photonic crystal operating around 1064 nm and its second harmonic at 532 nm. Indeed, a very powerful solid-state laser that can blind or destroy optical sensors and is widely available and easy to handle. In this work, we perform design and optimization by numerical simulations to determine the better structure for the nonlinear photonic crystal to achieve compact and efficient integrated optical limiter. The approach consists to analyze the band structures in Kerr-nonlinear two-dimensional photonic crystals as a function of the optical intensity. We confirm that these bands are dynamically red-shifted with regard to the bands observed in linear photonic crystals or in the case of weak nonlinear effects. The implemented approach will help to understand such phenomena as intensitydriven optical limiting with Kerr-nonlinear photonic crystals.

  3. Role of dynamical screening in excitation kinetics of biased quantum wells: Nonlinear absorption and ultrabroadband terahertz emission

    DEFF Research Database (Denmark)

    Turchinovich, Dmitry; Monozon, B. S.; Jepsen, Peter Uhd

    2006-01-01

    calculations, in particular, predict the strongly nonlinear dependency of the effective optical absorption coefficient on the excitation pulse fluence, and ultrabroadband terahertz emission. Our theoretical model is free of fitting parameters. Calculations performed for internally biased InFaN/GaN quantum...

  4. Quantum annealing with all-to-all connected nonlinear oscillators

    DEFF Research Database (Denmark)

    Puri, Shruti; Andersen, Christian Kraglund; Grimsmo, Arne L.

    2017-01-01

    Quantum annealing aims at solving combinatorial optimization problems mapped to Ising interactions between quantum spins. Here, with the objective of developing a noise-resilient annealer, we propose a paradigm for quantum annealing with a scalable network of two-photon-driven Kerr......-nonlinear resonators. Each resonator encodes an Ising spin in a robust degenerate subspace formed by two coherent states of opposite phases. A fully connected optimization problem is mapped to local fields driving the resonators, which are connected with only local four-body interactions. We describe an adiabatic...... annealing protocol in this system and analyse its performance in the presence of photon loss. Numerical simulations indicate substantial resilience to this noise channel, leading to a high success probability for quantum annealing. Finally, we propose a realistic circuit QED implementation of this promising...

  5. Self-similar asymptotic optical beams in semiconductor waveguides doped with quantum dots

    Science.gov (United States)

    He, Jun-Rong; Yi, Lin; Li, Hua-Mei

    2017-01-01

    The self-similar propagation of asymptotic optical beams in semiconductor waveguides doped with quantum dots is reported. The possibility of controlling the shape of output asymptotic optical beams is demonstrated. The analytical results are confirmed by numerical simulations. We give a possible experimental protocol to generate the obtained asymptotic parabolic beams in realistic waveguides. As a generalization to the present work, the self-similar propagation of asymptotic optical beams is proposed in a power-law nonlinear medium.

  6. Large optical nonlinearity of indium tin oxide in its epsilon-near-zero region.

    Science.gov (United States)

    Alam, M Zahirul; De Leon, Israel; Boyd, Robert W

    2016-05-13

    Nonlinear optical phenomena are crucial for a broad range of applications, such as microscopy, all-optical data processing, and quantum information. However, materials usually exhibit a weak optical nonlinearity even under intense coherent illumination. We report that indium tin oxide can acquire an ultrafast and large intensity-dependent refractive index in the region of the spectrum where the real part of its permittivity vanishes. We observe a change in the real part of the refractive index of 0.72 ± 0.025, corresponding to 170% of the linear refractive index. This change in refractive index is reversible with a recovery time of about 360 femtoseconds. Our results offer the possibility of designing material structures with large ultrafast nonlinearity for applications in nanophotonics. Copyright © 2016, American Association for the Advancement of Science.

  7. Tamper-indicating quantum optical seals

    Energy Technology Data Exchange (ETDEWEB)

    Humble, Travis S [ORNL; Williams, Brian P [ORNL

    2015-01-01

    Confidence in the means for identifying when tampering occurs is critical for containment and surveillance technologies. Fiber-optic seals have proven especially useful for actively surveying large areas or inventories due to the extended transmission range and flexible layout of fiber. However, it is reasonable to suspect that an intruder could tamper with a fiber-optic sensor by accurately replicating the light transmitted through the fiber. In this contribution, we demonstrate a novel approach to using fiber-optic seals for safeguarding large-scale inventories with increased confidence in the state of the seal. Our approach is based on the use of quantum mechanical phenomena to offer unprecedented surety in the authentication of the seal state. In particular, we show how quantum entangled photons can be used to monitor the integrity of a fiber-optic cable - the entangled photons serve as active sensing elements whose non-local correlations indicate normal seal operation. Moreover, we prove using the quantum no-cloning theorem that attacks against the quantum seal necessarily disturb its state and that these disturbances are immediately detected. Our quantum approach to seal authentication is based on physical principles alone and does not require the use of secret or proprietary information to ensure proper operation. We demonstrate an implementation of the quantum seal using a pair of entangled photons and we summarize our experimental results including the probability of detecting intrusions and the overall stability of the system design. We conclude by discussing the use of both free-space and fiber-based quantum seals for surveying large areas and inventories.

  8. Nonlinear super-resolution nano-optics and applications

    CERN Document Server

    Wei, Jingsong

    2015-01-01

    This book covers many advances in the subjects of nano-optics and nano photonics. The author describes the principle and technical schematics of common methods for breaking through the optical diffraction limit and focuses on realizing optical super-resolution with nonlinear effects of thin film materials. The applications of nonlinear optical super-resolution effects in nano-data storage, nanolithography, and nano-imaging are also presented. This book is useful to graduate students majoring in optics and nano science and also serves as a reference book for academic researchers, engineers, technical professionals in the fields of super-resolution optics and laser techniques, nano-optics and nano photonics, nano-data storage, nano imaging, micro/nanofabrication and nanolithography and nonlinear optics.

  9. Improved fiber nonlinearity mitigation in dispersion managed optical OFDM links

    Science.gov (United States)

    Tamilarasan, Ilavarasan; Saminathan, Brindha; Murugappan, Meenakshi

    2017-02-01

    Fiber nonlinearity is seen as a capacity limiting factor in OFDM based dispersion managed links since the Four Wave Mixing effects become enhanced due to the high PAPR. In this paper, the authors have compared the linear and nonlinear PAPR reduction techniques for fiber nonlinearity mitigation in OFDM based dispersion managed links. In the existing optical systems, linear transform techniques such as SLM and PTS have been implemented to reduce nonlinear effects. In the proposed study, superior performance of the L2-by-3 nonlinear transform technique is demonstrated for PAPR reduction to mitigate fiber nonlinearities. The performance evaluation is carried out by interfacing multiple simulators. The results of both linear and nonlinear transform techniques have been compared and the results show that nonlinear transform technique outperforms the linear transform in terms of nonlinearity mitigation and improved BER performance.

  10. Nonlinear optical properties of Au/PVP composite thin films

    Institute of Scientific and Technical Information of China (English)

    Shen Hong; Cheng Bo-Lin; Lu Guo-Wei; Wang Wei-Tian; Guan Dong-Yi; Chen Zheng-Hao; Yang Guo-Zhen

    2005-01-01

    Colloidal Au and poly(vinylpyrrolidone) (PVP) composite thin films are fabricated by spin-coating method. Linear optical absorption measurements of the Au/PVP composite films indicate an absorption peak around 530 nm due to the surface plasmon resonance of gold nanoparticles. Nonlinear optical properties are studied using standard Z-scan technique, and experimental results show large optical nonlinearities of the Au/PVP composite films. A large value of films.

  11. Quantum phases in optical lattices

    NARCIS (Netherlands)

    Dickerscheid, Dennis Brian Martin

    2006-01-01

    An important new development in the field of ultracold atomic gases is the study of the properties of these gases in a so-called optical lattice. An optical lattice is a periodic trapping potential for the atoms that is formed by the interference pattern of a few laser beams. A reason for the

  12. Theory of Electro-optic Modulation via a Quantum Dot Coupled to a Nano-resonator

    CERN Document Server

    Majumdar, Arka; Faraon, Andrei; Vuckovic, Jelena

    2009-01-01

    In this paper, we analyze the performance of an electro-optic modulator based on a single quantum dot strongly coupled to a nano-resonator, where electrical control of the quantum dot frequency is achieved via quantum confined Stark effect. Using realistic system parameters, we show that modulation speeds of a few tens of GHz are achievable with this system, while the energy per switching operation can be as small as 0.5 fJ. In addition, we study the non-linear distortion, and the effect of pure quantum dot dephasing on the performance of the modulator.

  13. Topics in linear optical quantum computation

    Science.gov (United States)

    Glancy, Scott Charles

    This thesis covers several topics in optical quantum computation. A quantum computer is a computational device which is able to manipulate information by performing unitary operations on some physical system whose state can be described as a vector (or mixture of vectors) in a Hilbert space. The basic unit of information, called the qubit, is considered to be a system with two orthogonal states, which are assigned logical values of 0 and 1. Photons make excellent candidates to serve as qubits. They have little interactions with the environment. Many operations can be performed using very simple linear optical devices such as beam splitters and phase shifters. Photons can easily be processed through circuit-like networks. Operations can be performed in very short times. Photons are ideally suited for the long-distance communication of quantum information. The great difficulty in constructing an optical quantum computer is that photons naturally interact weakly with one another. This thesis first gives a brief review of two early approaches to optical quantum computation. It will describe how any discrete unitary operation can be performed using a single photon and a network of beam splitters, and how the Kerr effect can be used to construct a two photon logic gate. Second, this work provides a thorough introduction to the linear optical quantum computer developed by Knill, Laflamme, and Milburn. It then presents this author's results on the reliability of this scheme when implemented using imperfect photon detectors. This author finds that quantum computers of this sort cannot be built using current technology. Third, this dissertation describes a method for constructing a linear optical quantum computer using nearly orthogonal coherent states of light as the qubits. It shows how a universal set of logic operations can be performed, including calculations of the fidelity with which these operations may be accomplished. It discusses methods for reducing and

  14. Quantum optics shines in the photon's centenary

    CERN Multimedia

    Cho, Adrian

    2005-01-01

    Hundred years after Einstein's hypothesis, the 2005 Nobel Prize in physics honors three researchers who have pioneered the frontier between the wave and particle views of light and laid the foundation for the field of "quantum optics" (1/2 page)

  15. Saturating optical resonances in quantum dots

    Science.gov (United States)

    Nair, Selvakumar V.; Rustagi, K. C.

    Optical bistability in quantum dots, recently proposed by Chemla and Miller, is studied in a two-resonance model. We show that for such classical electromagnetic resonances the applicability of a two-resonance model is far more restrictive than for those in atoms.

  16. Nonlinear Optical Materials for the Smart Filtering of Optical Radiation.

    Science.gov (United States)

    Dini, Danilo; Calvete, Mário J F; Hanack, Michael

    2016-11-23

    The control of luminous radiation has extremely important implications for modern and future technologies as well as in medicine. In this Review, we detail chemical structures and their relevant photophysical features for various groups of materials, including organic dyes such as metalloporphyrins and metallophthalocyanines (and derivatives), other common organic materials, mixed metal complexes and clusters, fullerenes, dendrimeric nanocomposites, polymeric materials (organic and/or inorganic), inorganic semiconductors, and other nanoscopic materials, utilized or potentially useful for the realization of devices able to filter in a smart way an external radiation. The concept of smart is referred to the characteristic of those materials that are capable to filter the radiation in a dynamic way without the need of an ancillary system for the activation of the required transmission change. In particular, this Review gives emphasis to the nonlinear optical properties of photoactive materials for the function of optical power limiting. All known mechanisms of optical limiting have been analyzed and discussed for the different types of materials.

  17. Optical and Nonlinear Optical Response of Light Sensor Thin Films

    Directory of Open Access Journals (Sweden)

    S. Z. Weisz

    2005-04-01

    Full Text Available For potential ultrafast optical sensor application, both VO2 thin films andnanocomposite crystal-Si enriched SiO2 thin films grown on fused quartz substrates weresuccessfully prepared using pulsed laser deposition (PLD and RF co-sputteringtechniques. In photoluminescence (PL measurement c-Si/SiO2 film containsnanoparticles of crystal Si exhibits strong red emission with the band maximum rangingfrom 580 to 750 nm. With ultrashort pulsed laser excitation all films show extremelyintense and ultrafast nonlinear optical (NLO response. The recorded holography fromall these thin films in a degenerate-four-wave-mixing configuration shows extremelylarge third-order response. For VO2 thin films, an optically induced semiconductor-tometalphase transition (PT immediately occurred upon laser excitation. it accompanied.It turns out that the fast excited state dynamics was responsible to the induced PT. For c-Si/SiO2 film, its NLO response comes from the contribution of charge carriers created bylaser excitation in conduction band of the c-Si nanoparticles. It was verified byintroducing Eu3+ which is often used as a probe sensing the environment variations. Itturns out that the entire excited state dynamical process associated with the creation,movement and trapping of the charge carriers has a characteristic 500 ps duration.

  18. Topology optimization of nonlinear optical devices

    DEFF Research Database (Denmark)

    Jensen, Jakob Søndergaard

    2011-01-01

    This paper considers the design of nonlinear photonic devices. The nonlinearity stems from a nonlinear material model with a permittivity that depends on the local time-averaged intensity of the electric field. A finite element model is developed for time-harmonic wave propagation and an incremen......This paper considers the design of nonlinear photonic devices. The nonlinearity stems from a nonlinear material model with a permittivity that depends on the local time-averaged intensity of the electric field. A finite element model is developed for time-harmonic wave propagation...

  19. Rate equations model and optical external efficiency of optically pumped electrically driven terahertz quantum cascade lasers

    Science.gov (United States)

    Hamadou, A.; Thobel, J.-L.; Lamari, S.

    2016-10-01

    A four level rate equations model for a terahertz optically pumped electrically driven quantum cascade laser is here introduced and used to model the system both analytically and numerically. In the steady state, both in the presence and absence of the terahertz optical field, we solve the resulting nonlinear system of equations and obtain closed form expressions for the levels occupation, population inversion as well as the mid-infrared pump threshold intensity in terms of the device parameters. We also derive, for the first time for this system, an analytical formula for the optical external efficiency and analyze the simultaneous effects of the cavity length and pump intensity on it. At moderate to high pump intensities, we find that the optical external efficiency scales roughly as the reciprocal of the cavity length.

  20. Quantum information processing with optical vortices

    Energy Technology Data Exchange (ETDEWEB)

    Khoury, Antonio Z. [Universidade Federal Fluminense (UFF), Niteroi, RJ (Brazil)

    2012-07-01

    Full text: In this work we discuss several proposals for quantum information processing using the transverse structure of paraxial beams. Different techniques for production and manipulation of optical vortices have been employed and combined with polarization transformations in order to investigate fundamental properties of quantum entanglement as well as to propose new tools for quantum information processing. As an example, we have recently proposed and demonstrated a controlled NOT (CNOT) gate based on a Michelson interferometer in which the photon polarization is the control bit and the first order transverse mode is the target. The device is based on a single lens design for an astigmatic mode converter that transforms the transverse mode of paraxial optical beams. In analogy with Bell's inequality for two-qubit quantum states, we propose an inequality criterion for the non-separability of the spin-orbit degrees of freedom of a laser beam. A definition of separable and non-separable spin-orbit modes is used in consonance with the one presented in Phys. Rev. Lett. 99, 2007. As the usual Bell's inequality can be violated for entangled two-qubit quantum states, we show both theoretically and experimentally that the proposed spin-orbit inequality criterion can be violated for non-separable modes. The inequality is discussed both in the classical and quantum domains. We propose a polarization to orbital angular momentum teleportation scheme using entangled photon pairs generated by spontaneous parametric down conversion. By making a joint detection of the polarization and angular momentum parity of a single photon, we are able to detect all the Bell-states and perform, in principle, perfect teleportation from a discrete to a continuous system using minimal resources. The proposed protocol implementation demands experimental resources that are currently available in quantum optics laboratories. (author)

  1. Entanglement Dynamics of Quantum Oscillators Nonlinearly Coupled to Thermal Environments

    OpenAIRE

    Voje, Aurora; Croy, Alexander; Isacsson, Andreas

    2014-01-01

    We study the asymptotic entanglement of two quantum harmonic oscillators nonlinearly coupled to an environment. Coupling to independent baths and a common bath are investigated. Numerical results obtained using the Wangsness-Bloch-Redfield method are supplemented by analytical results in the rotating wave approximation. The asymptotic negativity as function of temperature, initial squeezing and coupling strength, is compared to results for systems with linear system-reservoir coupling. We fin...

  2. Quantum metamaterials in the microwave and optical ranges

    CERN Document Server

    Zagoskin, A M; Rousseau, Emmanuel

    2016-01-01

    Quantum metamaterials generalize the concept of metamaterials (artificial optical media) to the case when their optical properties are determined by the interplay of quantum effects in the constituent 'artificial atoms' with the electromagnetic field modes in the system. The theoretical investigation of these structures demonstrated that a number of new effects (such as quantum birefringence, strongly nonclassical states of light, etc) are to be expected, prompting the efforts on their fabrication and experimental investigation. Here we provide a summary of the principal features of quantum metamaterials and review the current state of research in this quickly developing field, which bridges quantum optics, quantum condensed matter theory and quantum information processing.

  3. Nonlinear and Dispersive Optical Pulse Propagation

    Science.gov (United States)

    Dijaili, Sol Peter

    In this dissertation, there are basically four novel contributions to the field of picosecond pulse propagation and measurement. The first contribution is the temporal ABCD matrix which is an analog of the traditional ABCD ray matrices used in Gaussian beam propagation. The temporal ABCD matrix allows for the easy calculation of the effects of linear chirp or group velocity dispersion in the time domain. As with Gaussian beams in space, there also exists a complete Hermite-Gaussian basis in time whose propagation can be tracked with the temporal ABCD matrices. The second contribution is the timing synchronization between a colliding pulse mode-locked dye laser and a gain-switched Fabry-Perot type AlGaAs laser diode that has achieved less than 40 femtoseconds of relative timing jitter by using a pulsed optical phase lock loop (POPLL). The relative timing jitter was measured using the error voltage of the feedback loop. This method of measurement is accurate since the frequencies of all the timing fluctuations fall within the loop bandwidth. The novel element is a broad band optical cross-correlator that can resolve femtosecond time delay errors between two pulse trains. The third contribution is a novel dispersive technique of determining the nonlinear frequency sweep of a picosecond pulse with relatively good accuracy. All the measurements are made in the time domain and hence there is no time-bandwidth limitation to the accuracy. The fourth contribution is the first demonstration of cross -phase modulation in a semiconductor laser amplifier where a variable chirp was observed. A simple expression for the chirp imparted on a weak signal pulse by the action of a strong pump pulse is derived. A maximum frequency excursion of 16 GHz due to the cross-phase modulation was measured. A value of 5 was found for alpha _{xpm} which is a factor for characterizing the cross-phase modulation in a similar manner to the conventional linewidth enhancement factor, alpha.

  4. Linear and nonlinear optical properties of chalcogenide microstructured optical fibers

    Science.gov (United States)

    Trolès, Johann; Brilland, Laurent; Caillaud, Celine; Renversez, Gilles; Mechin, David; Adam, Jean-Luc

    2015-03-01

    Chalcogenide glasses are known for their large transparency in the mid-infrared and their high linear refractive index (>2). They present also a high non-linear coefficient (n2), 100 to 1000 times larger than for silica, depending on the composition. we have developed a casting method to prepare the microstructured chalcogenide preform. This method allows optical losses as low as 0.4 dB/m at 1.55 µm and less than 0.05 dB/m in the mid IR. Various chalcogenide MOFs operating in the IR range has been fabricated in order to associate the high non-linear properties of these glasses and the original MOF properties. For example, small core fibers have been drawn to enhance the non linearities for telecom applications such as signal regeneration and generation of supercontinuum sources. On another hand, in the 3-12 µm window, single mode fibers and exposed core fibers have been realized for Gaussian beams propagation and sensors applications respectively.

  5. Nonlinear optical properties of manganese porphyrin-incorporated PVC film

    Directory of Open Access Journals (Sweden)

    Jeong-Hyon Ha

    2010-12-01

    Full Text Available We measured thermally originated solid phase nonlinear optical properties of manganese porphyrin-incorporated PVC polymer film using CW low-power Z-scan and optical power limiting methods. The nonlinear refractive index (n2 of this porphyrin film is estimated to have a negative value of 7.2 ⅹ10-5 cm2/W at 632.8 nm and to be larger than that of ZnTPP in the Nafion film. The photodegradation effect common in the solution phase appears to be minor in this solid phase system. The large nonlinear effect is thought to limit the optical power due to the aperture effect.

  6. Nonlinear optical microscopy for imaging thin films and surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Smilowitz, L.B.; McBranch, D.W.; Robinson, J.M.

    1995-03-01

    We have used the inherent surface sensitivity of second harmonic generation to develop an instrument for nonlinear optical microscopy of surfaces and interfaces. We have demonstrated the use of several nonlinear optical responses for imaging thin films. The second harmonic response of a thin film of C{sub 60} has been used to image patterned films. Two photon absorption light induced fluorescence has been used to image patterned thin films of Rhodamine 6G. Applications of nonlinear optical microscopy include the imaging of charge injection and photoinduced charge transfer between layers in semiconductor heterojunction devices as well as across membranes in biological systems.

  7. Population Dynamics and the Optical Absorption in Hybrid Metal Nanoparticle - Semiconductor Quantum dot Nanosystem

    CERN Document Server

    Kim, Nam-Chol; Ko, Myong-Chol; So, Guang Hyok; Kim, Il-Guang

    2015-01-01

    We studied theoretically the population dynamics and the absorption spectrum of hybrid nanosystem consisted of a matal nanoparticle (MNP) and a semiconductor quantum dot(SQD). We investigated the exciton-plasmon coupling effects on the population dynamics and the absorption properties of the nanostructure. Our results show that the nonlinear optical response of the hybrid nanosystem can be greatly enhanced or depressed due to the exciton-plasmon couplings. The results obtained here may have the potential applications of nanoscale optical devices such as optical switches and quantum devices such as a single photon transistor.

  8. Interplay between dissipation and driving in nonlinear quantum systems

    Energy Technology Data Exchange (ETDEWEB)

    Vierheilig, Carmen

    2011-07-01

    In this thesis we investigate the interplay between dissipation and driving in nonlinear quantum systems for a special setup: a flux qubit read out by a DC-SQUID - a nonlinear quantum oscillator. The latter is embedded in a harmonic bath, thereby mediating dissipation to the qubit. Two different approaches are elaborated: First we consider a composite qubit-SQUID system and add the bath afterwards. We derive analytical expressions for its eigenstates beyond rotating wave approximation (RWA), by applying Van Vleck perturbation theory (VVPT) in the qubit-oscillator coupling. The second approach is an effective bath approach based on a mapping procedure, where SQUID and bath form an effective bath seen by the qubit. Here the qubit dynamics is obtained by applying standard procedures established for the spin-boson problem. This approach requires the knowledge of the steady-state response of the dissipative Duffing oscillator, which is studied within a resonant and an offresonant approach: The first is applicable near and at an N-photon resonance using VVPT beyond a RWA. The second is based on the exact Floquet states of the nonlinear driven oscillator. The dissipative qubit dynamics is described analytically for weak system-bath coupling and agrees well for both approaches. We derive the effect of the nonlinearity on the qubit dynamics, on the Bloch-Siegert shift and on the vacuum Rabi splitting. (orig.)

  9. Modeling and compensation of transmitter nonlinearity in coherent optical OFDM.

    Science.gov (United States)

    Amiralizadeh, Siamak; Nguyen, An T; Rusch, Leslie A

    2015-10-05

    We present a comprehensive study of nonlinear distortions from an optical OFDM transmitter. Nonlinearities are introduced by the combination of effects from the digital-to-analog converter (DAC), electrical power amplifier (PA) and optical modulator in the presence of high peak-to-average power ratio (PAPR). We introduce parameters to quantify the transmitter nonlinearity. High input backoff avoids OFDM signal compression from the PA, but incurs high penalties in power efficiency. At low input backoff, common PAPR reduction techniques are not effective in suppressing the PA nonlinear distortion. A bit error distribution investigation shows a technique combining nonlinear predistortion with PAPR mitigation could achieve good power efficiency by allowing low input backoff. We use training symbols to extract the transmitter nonlinear function. We show that piecewise linear interpolation (PLI) leads to an accurate transmitter nonlinearity characterization. We derive a semi-analytical solution for bit error rate (BER) that validates the PLI approximation accurately captures transmitter nonlinearity. The inverse of the PLI estimate of the nonlinear function is used as a predistorter to suppress transmitter nonlinearity. We investigate performance of the proposed scheme by Monte Carlo simulations. Our simulations show that when DAC resolution is more than 4 bits, BER below forward error correction limit of 3.8 × 10(-3) can be achieved by using predistortion with very low input power backoff for electrical PA and optical modulator.

  10. Chip scale low dimensional materials: optoelectronics & nonlinear optics

    Science.gov (United States)

    Gu, Tingyi

    The CMOS foundry infrastructure enables integration of high density, high performance optical transceivers. We developed integrated devices that assemble resonators, waveguide, tapered couplers, pn junction and electrodes. Not only the volume standard manufacture in silicon foundry is promising to low-lost optical components operating at IR and mid-IR range, it also provides a robust platform for revealing new physical phenomenon. The thesis starts from comparison between photonic crystal and micro-ring resonators based on chip routers, showing photonic crystal switches have small footprint, consume low operation power, but its higher linear loss may require extra energy for signal amplification. Different designs are employed in their implementation in optical signal routing on chip. The second part of chapter 2 reviews the graphene based optoelectronic devices, such as modulators, lasers, switches and detectors, potential for group IV optoelectronic integrated circuits (OEIC). In chapter 3, the highly efficient thermal optic control could act as on-chip switches and (transmittance) tunable filters. Local temperature tuning compensates the wavelength differences between two resonances, and separate electrode is used for fine tuning of optical pathways between two resonators. In frequency domain, the two cavity system also serves as an optical analogue of Autler-Towns splitting, where the cavity-cavity resonance detuning is controlled by the length of pathway (phase) between them. The high thermal sensitivity of cavity resonance also effectively reflects the heat distribution around the nanoheaters, and thus derives the thermal conductivity in the planar porous suspended silicon membrane. Chapter 4 & 5 analyze graphene-silicon photonic crystal cavities with high Q and small mode volume. With negligible nonlinear response to the milliwatt laser excitation, the monolithic silicon PhC turns into highly nonlinear after transferring the single layer graphene with

  11. Modified Semi-Classical Methods for Nonlinear Quantum Oscillations Problems

    CERN Document Server

    Moncrief, Vincent; Maitra, Rachel

    2012-01-01

    We develop a modified semi-classical approach to the approximate solution of Schrodinger's equation for certain nonlinear quantum oscillations problems. At lowest order, the Hamilton-Jacobi equation of the conventional semi-classical formalism is replaced by an inverted-potential-vanishing-energy variant thereof. Under smoothness, convexity and coercivity hypotheses on its potential energy function, we prove, using the calculus of variations together with the Banach space implicit function theorem, the existence of a global, smooth `fundamental solution'. Higher order quantum corrections, for ground and excited states, are computed through the integration of associated systems of linear transport equations, and formal expansions for the corresponding energy eigenvalues obtained by imposing smoothness on the quantum corrections to the eigenfunctions. For linear oscillators our expansions naturally truncate, reproducing the well-known solutions for the energy eigenfunctions and eigenvalues. As an application, w...

  12. Nonlinear double Compton scattering in the full quantum regime

    CERN Document Server

    Mackenroth, F

    2012-01-01

    A detailed analysis of the process of two photon emission by an electron scattered from a high-intensity laser pulse is presented. The calculations are performed in the framework of strong-field QED and include exactly the presence of the laser field, described as a plane wave. We investigate the full quantum regime of interaction, where photon recoil plays an essential role in the emission process, and substantially alters the emitted photon spectra as compared to those in previously-studied regimes. We provide a semiclassical explanation for such differences, based on the possibility of assigning a trajectory to the electron in the laser field before and after each quantum photon emission. Our numerical results indicate the feasibility of investigating experimentally the full quantum regime of nonlinear double Compton scattering with already available plasma-based electron accelerator and laser technology.

  13. Quantum noise in large-scale coherent nonlinear photonic circuits

    CERN Document Server

    Santori, Charles; Beausoleil, Raymond G; Tezak, Nikolas; Hamerly, Ryan; Mabuchi, Hideo

    2014-01-01

    A semiclassical simulation approach is presented for studying quantum noise in large-scale photonic circuits incorporating an ideal Kerr nonlinearity. A netlist-based circuit solver is used to generate matrices defining a set of stochastic differential equations, in which the resonator field variables represent random samplings of the Wigner quasi-probability distributions. Although the semiclassical approach involves making a large-photon-number approximation, tests on one- and two-resonator circuits indicate satisfactory agreement between the semiclassical and full-quantum simulation results in the parameter regime of interest. The semiclassical model is used to simulate random errors in a large-scale circuit that contains 88 resonators and hundreds of components in total, and functions as a 4-bit ripple counter. The error rate as a function of on-state photon number is examined, and it is observed that the quantum fluctuation amplitudes do not increase as signals propagate through the circuit, an important...

  14. Quantum Dot Devices for Optical Signal Processing

    DEFF Research Database (Denmark)

    Chen, Yaohui

    . Additional to the static linear amplication properties, we focus on exploring the gain dynamics on the time scale ranging from sub-picosecond to nanosecond. In terms of optical signals that have been investigated, one is the simple sinusoidally modulated optical carrier with a typical modulation frequency...... range of 1-100 gigahertz. Our simulations reveal the role of ultrafast intradot carrier dynamics in enhancing modulation bandwidth of quantum dot semiconductor optical ampliers. Moreover, the corresponding coherent gain response also provides rich dispersion contents over a broad bandwidth. One...... important implementation is recently boosted by the research in slow light. The idea is to migrate such dynamical gain knowledge for the investigation of microwave phase shifter based on semiconductor optical waveguide. Our study reveals that phase shifting based on the conventional semiconductor optical...

  15. Instabilities in the optical response of a semiconductor quantum dot-metal nanoparticle heterodimer : self-oscillations and chaos

    NARCIS (Netherlands)

    Nugroho, Bintoro S.; Iskandar, Alexander A.; Malyshev, Victor A.; Knoester, Jasper

    We theoretically investigate the nonlinear optical response of a heterodimer comprising a semiconductor quantum dot strongly coupled to a metal nanoparticle. The quantum dot is considered as a three-level ladder system with ground, one-exciton, and bi-exction states. As compared to the case of a

  16. An optical analog of quantum optomechanics

    CERN Document Server

    Rodríguez-Lara, B M

    2014-01-01

    We present a two-dimensional array of nearest-neighbor coupled waveguides that is the optical analog of a quantum optomechanical system. We show that the quantum model predicts the appearance of effective column isolation, diagonal-coupling and other non-trivial couplings in the two-dimensional photonic lattice under a standard approximation from ion-trap cavity electrodynamics. We provide an approximate impulse function for the case of effective column isolation and compare it with exact numerical propagation in the photonic lattice.

  17. Controllable optical bistability and multistability in asymmetric double quantum wells via spontaneously generated coherence

    Energy Technology Data Exchange (ETDEWEB)

    Chen, Yuan; Deng, Li [Department of Applied Physics, East China Jiaotong University, Nanchang, 330013 (China); Chen, Aixi, E-mail: aixichen@ecjtu.jx.cn [Department of Applied Physics, East China Jiaotong University, Nanchang, 330013 (China); Institute for Quantum Computing, University of Waterloo, Ontario N2L 3G1 (Canada)

    2015-02-15

    We investigate the nonlinear optical phenomena of the optical bistability and multistability via spontaneously generated coherence in an asymmetric double quantum well structure coupled by a weak probe field and a controlling field. It is shown that the threshold and hysteresis cycle of the optical bistability can be conveniently controlled only by adjusting the intensity of the SGC or the controlling field. Moreover, switching between optical bistability and multistability can be achieved. These studies may have practical significance for the preparation of optical bistable switching device.

  18. Nonlinear photon-assisted tunneling transport in optical gap antennas.

    Science.gov (United States)

    Stolz, Arnaud; Berthelot, Johann; Mennemanteuil, Marie-Maxime; Colas des Francs, Gérard; Markey, Laurent; Meunier, Vincent; Bouhelier, Alexandre

    2014-05-14

    We introduce strongly coupled optical gap antennas to interface optical radiation with current-carrying electrons at the nanoscale. The transducer relies on the nonlinear optical and electrical properties of an optical gap antenna operating in the tunneling regime. We discuss the underlying physical mechanisms controlling the conversion involving d-band electrons and demonstrate that a simple two-wire optical antenna can provide advanced optoelectronic functionalities beyond tailoring the electromagnetic response of a single emitter. Interfacing an electronic command layer with a nanoscale optical device may thus be facilitated by the optical rectennas discussed here.

  19. Observation of nonlinear optical effects in some semiconductor quantum dot materials using Nd -' YAG laser radiation%半导体量子点材料在Nd:YAG激光辐照下的非线性光学效应

    Institute of Scientific and Technical Information of China (English)

    KUMBHAKAR P

    2011-01-01

    Nonlinear optical (NLO) properties of the colloidal solutions of chemically synthesized undoped and Mn2+ doped ZnS Quantum Dots (QDs) in methanol are measured by using a Q-switched 10 ns pulsed Nd: YAG laser radiation by the Z-scan technique. The nanostructures of the synthesized materials are characterized by using different characterization tools, such as Transmission Electron Microscopy (TEM) and X-ray Diffraction (XRD) analysis. Linear optical absorption and Photoluminescence (PL) emission characteristics of the colloidal solutions of the synthesized QDs are measured at room temperature by using a UV-visible spectrophotometer and a spectrofluorimeter, respectively.The absorption characteristics of the samples show that the absorption cut-off of the samples is below that of the bulk ZnS due to the quantum confinement effect. Photoluminescenee emission characteristics measured at room temperature show that the Mn2+ doped ZnS sample exhibits its visible PL emission peak at ~580 nm, whereas the undoped ZnS sample emits in the ultraviolet region peak at ~365 nm. The average particle size (radius) of the as-prepared ZnS sample is ~1. 2 nm as determined from the measured UV-visible absorption characteristics as well as from TEM and XRD data analyses. By analyzing the experimental data obtained by the Open Aperture (OA) Z-scan technique, it is found that the Four-photon Absorption (FPA) takes place at 1064 nm wavelength in both the studied samples. FPA coefficients and FPA cross-section of both the samples are extracted by fitting the experimental data with the available analytical expression. It is found that the calculated value of FPA cross section of ZnS QD is 4.9 × 10-106 cms · s3 · photon-3, which is five orders of magnitude larger than that of bulk ZnS. Optical limiting property of the synthesized ZnS QD is also presented. The simultaneous presence of large FPA cross section and large luminescence efficiency in the visible region in Mn2+ doped sample

  20. Electron quantum optics in ballistic chiral conductors

    Energy Technology Data Exchange (ETDEWEB)

    Bocquillon, Erwann; Freulon, Vincent; Parmentier, Francois D.; Berroir, Jean-Marc; Placais, Bernard; Feve, Gwendal [Laboratoire Pierre Aigrain, Ecole Normale Superieure, CNRS (UMR 8551), Universite Pierre et Marie Curie, Universite Paris Diderot, Paris (France); Wahl, Claire; Rech, Jerome; Jonckheere, Thibaut; Martin, Thierry [Aix Marseille Universite, CNRS, CPT, UMR 7332, Marseille (France); Universite de Toulon, CNRS, CPT, UMR 7332, La Garde (France); Grenier, Charles; Ferraro, Dario; Degiovanni, Pascal [Universite de Lyon, Federation de Physique Andre Marie Ampere, CNRS - Laboratoire de Physique de l' Ecole Normale Superieure de Lyon, Lyon (France)

    2014-01-15

    The edge channels of the quantum Hall effect provide one dimensional chiral and ballistic wires along which electrons can be guided in an optics-like setup. Electronic propagation can then be analyzed using concepts and tools derived from optics. After a brief review of electron optics experiments performed using stationary current sources which continuously emit electrons in the conductor, this paper focuses on triggered sources, which can generate on-demand a single particle state. It first outlines the electron optics formalism and its analogies and differences with photon optics and then turns to the presentation of single electron emitters and their characterization through the measurements of the average electrical current and its correlations. This is followed by a discussion of electron quantum optics experiments in the Hanbury-Brown and Twiss geometry where two-particle interferences occur. Finally, Coulomb interactions effects and their influence on single electron states are considered. (copyright 2013 by WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  1. Semiclassical theory of nonlinear magneto-optical responses with applications to topological Dirac/Weyl semimetals

    Science.gov (United States)

    Morimoto, Takahiro; Zhong, Shudan; Orenstein, Joseph; Moore, Joel E.

    2016-12-01

    We study nonlinear magneto-optical responses of metals by a semiclassical Boltzmann equation approach. We derive general formulas for linear and second-order nonlinear optical effects in the presence of magnetic fields that include both the Berry curvature and the orbital magnetic moment. Applied to Weyl fermions, the semiclassical approach (i) captures the directional anisotropy of linear conductivity under a magnetic field as a consequence of an anisotropic B2 contribution, which may explain the low-field regime of recent experiments; and (ii) predicts strong second harmonic generation proportional to B that is enhanced as the Fermi energy approaches the Weyl point, leading to large nonlinear Kerr rotation. Moreover, we show that the semiclassical formula for the circular photogalvanic effect arising from the Berry curvature dipole is reproduced by a full quantum calculation using a Floquet approach.

  2. Explicit formulation of second and third order optical nonlinearity in the FDTD framework

    CERN Document Server

    Varin, Charles; Bart, Graeme; Fennel, Thomas; Brabec, Thomas

    2016-01-01

    The finite-difference time-domain (FDTD) method is a flexible and powerful technique for rigorously solving Maxwell's equations. However, three-dimensional optical nonlinearity in current commercial and research FDTD softwares requires solving iteratively an implicit form of Maxwell's equations over the entire numerical space and at each time step. Reaching numerical convergence demands significant computational resources and practical implementation often implies a complete rewriting of the core FDTD engine. In this paper, we present an explicit method to include second and third order optical nonlinearity in the FDTD framework based on a nonlinear generalization of the Lorentz dispersion model derived from an analytical solution of the quantum mechanical two-level equations. With the proposed approach, numerical integration is simple, intuitive, fully explicit, and computationally efficient.

  3. Dielectric Optical-Controllable Magnifying Lens by Nonlinear Negative Refraction

    Science.gov (United States)

    Cao, Jianjun; Shang, Ce; Zheng, Yuanlin; Feng, Yaming; Chen, Xianfeng; Liang, Xiaogan; Wan, Wenjie

    2015-01-01

    A simple optical lens plays an important role for exploring the microscopic world in science and technology by refracting light with tailored spatially varying refractive indices. Recent advancements in nanotechnology enable novel lenses, such as, superlens and hyperlens, with sub-wavelength resolution capabilities by specially designed materials’ refractive indices with meta-materials and transformation optics. However, these artificially nano- or micro-engineered lenses usually suffer high losses from metals and are highly demanding in fabrication. Here, we experimentally demonstrate, for the first time, a nonlinear dielectric magnifying lens using negative refraction by degenerate four-wave mixing in a plano-concave glass slide, obtaining magnified images. Moreover, we transform a nonlinear flat lens into a magnifying lens by introducing transformation optics into the nonlinear regime, achieving an all-optical controllable lensing effect through nonlinear wave mixing, which may have many potential applications in microscopy and imaging science. PMID:26149952

  4. Extremely nonlocal optical nonlinearities in atoms trapped near a waveguide

    CERN Document Server

    Shahmoon, Ephraim; Stimming, Hans Peter; Mazets, Igor; Kurizki, Gershon

    2014-01-01

    Nonlinear optical phenomena are typically local. Here we predict the possibility of highly nonlocal optical nonlinearities for light propagating in atomic media trapped near a nano-waveguide, where long-range interactions between the atoms can be tailored. When the atoms are in an electromagnetically-induced transparency configuration, the atomic interactions are translated to long-range interactions between photons and thus to highly nonlocal optical nonlinearities. We derive and analyze the governing nonlinear propagation equation, finding a roton-like excitation spectrum for light and the emergence of long-range order in its output intensity. These predictions open the door to studies of unexplored wave dynamics and many-body physics with highly-nonlocal interactions of optical fields in one dimension.

  5. Dielectric Optical-Controlled Magnifying Lens by Nonlinear Negative Refraction

    CERN Document Server

    Cao, Jianjun; Zheng, Yuanlin; Chen, Xianfeng; Liang, Xiaogan; Wan, Wenjie

    2014-01-01

    A simple optical lens plays an important role for exploring the microscopic world in science and technology by refracting light with tailored spatially varying refractive index. Recent advancements in nanotechnology enable novel lenses, such as, superlens, hyperlens, Luneburg lens, with sub-wavelength resolution capabilities by specially designing materials' refractive indices with meta-materials and transformation optics. However, these artificially nano/micro engineered lenses usually suffer high losses from metals and are highly demanding in fabrication. Here we experimentally demonstrate for the first time a nonlinear dielectric magnifying lens using negative refraction by degenerate four-wave mixing in a plano-concave glass slide, obtaining magnified images. Moreover, we transform a nonlinear flat lens into a magnifying lens by introducing transformation optics into nonlinear regime, achieving an all-optical controllable lensing effect through nonlinear wave mixing, which may have many potential applicat...

  6. Intra-Channel Nonlinear Effect on Optical PPM Pulse Transmission

    Institute of Scientific and Technical Information of China (English)

    Sun; Linghao; Jarmo; Takala

    2003-01-01

    PPM encoded Gaussian pulse sequence shows more immunity than non-PPM schemes on optical fiber intra-channel nonlinearity and demonstrated by a numerical study of IXPM and IFWM effects deploying on 100Gb/s single channelsystem.

  7. Optical Nonlinearities in Chalcogenide Glasses and their Applications

    CERN Document Server

    Zakery, A

    2007-01-01

    Photonics, which uses photons for information and image processing, has been labeled the technology of the 21st century, for which non-linear optical processes provide the key functions of frequency conversion and optical switching. Chalcogenide glass fiber is one of the most promising candidates for use as a non-linear optical medium because of its high optical nonlinearity and long interaction length. Since the chalcogenide glass fibers transmit into the IR, there are numerous potential applications in the civil, medical and military areas. One of the most exciting developments in the future is going to be in the area of rare-earth ion doping of chalcogenide fibers for IR fluorescence emission. The IR light sources, lasers and amplifiers developed using this phenomena will be very useful in civil, medical and military applications. Remote IR spectroscopy and imaging using flexible fibers will be realized for applications. Other future research areas which will inevitably be explored includes non-linear opti...

  8. Topological nature of nonlinear optical effects in solids.

    Science.gov (United States)

    Morimoto, Takahiro; Nagaosa, Naoto

    2016-05-01

    There are a variety of nonlinear optical effects including higher harmonic generations, photovoltaic effects, and nonlinear Kerr rotations. They are realized by strong light irradiation to materials that results in nonlinear polarizations in the electric field. These are of great importance in studying the physics of excited states of the system as well as for applications to optical devices and solar cells. Nonlinear properties of materials are usually described by nonlinear susceptibilities, which have complex expressions including many matrix elements and energy denominators. On the other hand, a nonequilibrium steady state under an electric field periodic in time has a concise description in terms of the Floquet bands of electrons dressed by photons. We show theoretically, using the Floquet formalism, that various nonlinear optical effects, such as the shift current in noncentrosymmetric materials, photovoltaic Hall response, and photo-induced change of order parameters under the continuous irradiation of monochromatic light, can be described in a unified fashion by topological quantities involving the Berry connection and Berry curvature. We found that vector fields defined with the Berry connections in the space of momentum and/or parameters govern the nonlinear responses. This topological view offers a route to designing nonlinear optical materials.

  9. Merging Nonlinear Optics and Negative-Index Metamaterials

    CERN Document Server

    Popov, Alexander K

    2011-01-01

    The extraordinary properties of nonlinear optical propagation processes in double-domain positive/negative index metamaterials are reviewed. These processes include second harmonic generation, three- and four-wave frequency mixing, and optical parametric amplification. Striking contrasts with the properties of the counterparts in ordinary materials are shown. We also discuss the possibilities for compensating strong losses inherent to plasmonic metamaterials, which present a major obstacle in numerous exciting applications, and the possibilities for creation of unique ultracompact photonic devices such as data processing chips and nonlinear-optical sensors. Finally, we propose similar extraordinary three-wave mixing processes in crystals based on optical phonons with negative dispersion.

  10. Molecular and crystal design of nonlinear optical organic materials

    Energy Technology Data Exchange (ETDEWEB)

    Suponitsky, Kirill Yu; Antipin, Mikhail Yu [A.N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Moscow (Russian Federation); Timofeeva, Tatiana V [Department of Chemistry, New Mexico Highlands University (United States)

    2006-06-30

    The results of theoretical and experimental studies on the second-order molecular and crystal nonlinear optical susceptibilities of organic and several classes of organoelement compounds are summarised. Modern methods used in these studies are briefly characterised, their advantages and drawbacks are outlined as regards their application to the systematic search for efficient nonlinear optical materials. Recent achievements and the main challenges in the field are thoroughly discussed and an optimum algorithm of the design of such materials is proposed.

  11. Photonic nanowires for quantum optics

    DEFF Research Database (Denmark)

    Munsch, M.; Claudon, J.; Bleuse, J.;

    Photonic nanowires (PWs) are simple dielectric structures for which a very efficient and broadband spontaneous emission (SE) control has been predicted [1]. Recently, a single photon source featuring a record high efficiency was demonstrated using this geometry [2]. Using time-resolved micro......-photoluminescence, we investigate directly the SE of single InAs quantum dots (QDs) embedded in GaAs PWs and demonstrate performances that fully confirm the theoretical predictions [3]. In addition, we discuss recent results obtained on elliptical wires that ensure an efficient control of the photon polarization [4......, equivalent to the one obtained in state-of-the-art 2D photonic crystals, is measured. Moreover, a PW featuring an elliptical section provides a very efficient control over the polarization of the emitted photon. In that case, only one guided mode, with a linear polarization oriented along the major axis...

  12. Beyond Quantum interference and Optical pumping: invoking a Closed-loop phase

    CERN Document Server

    Kani, A

    2016-01-01

    Atomic coherence effects arising from coherent light-atom interaction are conventionally known to be governed by quantum interference and optical pumping mechanisms. However, anisotropic nonlinear response driven by optical field involves another fundamental effect arising from closed-loop multiphoton transitions. This closed-loop phase dictates the tensorial structure of the nonlinear susceptibility as it governs the principal coordinate system in determining, whether the light field will either compete or cooperate with the external magnetic field stimulus. Such a treatment provides deeper understanding of all magneto-optical anisotropic response. The magneto-optical response in all atomic systems is classified using closed-loop phase. The role of quantum interference in obtaining electromagnetically induced transparency or electromagnetically induced absorption in multi-level systems is identified.

  13. Improvement of nonlinear optical properties of graphene oxide in mixed with Ag2S@ZnS core-shells

    Science.gov (United States)

    Khanzadeh, M.; Dehghanipour, M.; Karimipour, M.; Molaei, M.

    2017-04-01

    Nonlinear optical properties including size and sign of nonlinear refractive index and nonlinear absorption coefficient of Graphene Oxide (GO), Ag2S@ZnS quantum dots and GO-Ag2S@ZnS were investigated using a Z-scan technique by laser diode with 532 nm wavelength. Third-order susceptibility of the compounds was calculated and compared with the reported values. By comparing the nonlinear optical (NLO) properties of GO and the mixture of GO-Ag2S@ZnS, it was observed that the NLO properties of GO were increased using simply mixing with Ag2S@ZnS quantum dots. It was also observed that with increase of sonication time, the NLO properties of the mixture increased accordingly.

  14. Frames and fusion frames in quantum optics

    Energy Technology Data Exchange (ETDEWEB)

    Jamiolkowski, Andrzej, E-mail: jam@fizyka.umk.p [Institute of Physics, Nicholas Copernicus University, 87-100 Torun (Poland)

    2010-03-01

    The main purpose of this paper is to show that the notions of frames and fusion frames introduced in non-harmonic Fourier analysis are also very natural in discussion of some basic problems in theory of open quantum systems and, in particular, in quantum optics. Frames are collections of vectors in a Hilbert space which assure a natural representation of each vector in the space, but may have infinitely many different representations for any given vector. For a given quantum system represented in a Hilbert space H the question of minimal number {eta} of observables Q{sub 1},..., Q{sub {eta}} whose expectation values at some instants t{sub 1},...,t{sub p} determine the statistical state of the system is discussed. We assume that the time evolution of the system in question is governed by a semigroup of linear transformations with generator L.

  15. Optical computation based on nonlinear total reflectional optical switch at the interface

    Indian Academy of Sciences (India)

    Jianqi Zhang; Huan Xu

    2009-03-01

    A new scheme of binary half adder and full adder is proposed. It realizes a kind of all-optical computation which is based on the polarization coding technique and the nonlinear total reflectional optical switches.

  16. Fiber-Optic Sources of Quantum Entanglement

    CERN Document Server

    Kumar, P; Fiorentino, M; Voss, P L; Sharping, J E; Barbosa, G A

    2002-01-01

    We present a fiber-based source of polarization-entangled photon pairs that is well suited for quantum communication applications in the 1.5$\\mu$m band of standard telecommunication fiber. Quantum-correlated signal and idler photon pairs are produced when a nonlinear-fiber Sagnac interferometer is pumped in the anomalous-dispersion region of the fiber. Recently, we have demonstrated nonclassical properties of such photon pairs by using Geiger-mode InGaAs/InP avalanche photodiodes. Polarization entanglement in the photon pairs can be created by pumping the Sagnac interferometer with two orthogonally polarized pulses. In this case the parametrically scattered signal-idler photons yield biphoton interference with $>$90% visibility in coincidence detection, while no interference is observed in direct detection of either the signal or the idler photons.

  17. Integrated Quantum Optics: Experiments towards integrated quantum-light sources and quantum-enhanced sensing

    DEFF Research Database (Denmark)

    Hoff, Ulrich Busk

    The work presented in this thesis is focused on experimental application and generation of continuous variable quantum correlated states of light in integrated dielectric structures. Squeezed states are among the most exploited continuous variable optical states for free-space quantum-enhanced se......The work presented in this thesis is focused on experimental application and generation of continuous variable quantum correlated states of light in integrated dielectric structures. Squeezed states are among the most exploited continuous variable optical states for free-space quantum...... in this thesis: Firstly, we present proof-of-principle demonstration of interfacing squeezed light with an on-chip optomechanical resonator, demonstrating a quantum-enhanced sensitivity to the vibrations of the micromechanical object. Secondly, work on developing an integrated source of squeezed light...

  18. New CMOS Compatible Platforms for Integrated Nonlinear Optical Signal Processing

    CERN Document Server

    Moss, D J

    2014-01-01

    Nonlinear photonic chips have succeeded in generating and processing signals all-optically with performance far superior to that possible electronically - particularly with respect to speed. Although silicon-on-insulator has been the leading platform for nonlinear optics, its high two-photon absorption at telecommunications wavelengths poses a fundamental limitation. This paper reviews some of the recent achievements in CMOS-compatible platforms for nonlinear optics, focusing on amorphous silicon and Hydex glass, highlighting their potential future impact as well as the challenges to achieving practical solutions for many key applications. These material systems have opened up many new capabilities such as on-chip optical frequency comb generation and ultrafast optical pulse generation and measurement.

  19. Platforms for integrated nonlinear optics compatible with silicon integrated circuits

    CERN Document Server

    Moss, David J

    2014-01-01

    Nonlinear photonic chips are capable of generating and processing signals all-optically with performance far superior to that possible electronically - particularly with respect to speed. Although silicon has been the leading platform for nonlinear optics, its high two-photon absorption at telecommunications wavelengths poses a fundamental limitation. We review recent progress in CMOS-compatible platforms for nonlinear optics, focusing on Hydex glass and silicon nitride and briefly discuss the promising new platform of amorphous silicon. These material systems have opened up many new capabilities such as on-chip optical frequency comb generation, ultrafast optical pulse generation and measurement. We highlight their potential future impact as well as the challenges to achieving practical solutions for many key applications.

  20. Distributed quantum computation via optical fibres

    CERN Document Server

    Serafini, A; Bose, S; Serafini, Alessio; Mancini, Stefano; Bose, Sougato

    2005-01-01

    We investigate the possibility of realising effective quantum gates between two atoms in distant cavities coupled by an optical fibre. We show that highly reliable swap and entangling gates are achievable. We exactly study the stability of these gates in presence of imperfections in coupling strengths and interaction times and prove them to be robust. Moreover, we analyse the effect of spontaneous emission and losses and show that such gates are very promising in view of the high level of coherent control currently achievable in optical cavities.