Nonlinear optical interactions in silicon waveguides
Directory of Open Access Journals (Sweden)
Kuyken B.
2017-03-01
Full Text Available The strong nonlinear response of silicon photonic nanowire waveguides allows for the integration of nonlinear optical functions on a chip. However, the detrimental nonlinear optical absorption in silicon at telecom wavelengths limits the efficiency of many such experiments. In this review, several approaches are proposed and demonstrated to overcome this fundamental issue. By using the proposed methods, we demonstrate amongst others supercontinuum generation, frequency comb generation, a parametric optical amplifier, and a parametric optical oscillator.
International Nuclear Information System (INIS)
Boyd, R.W.
1992-01-01
Nonlinear optics is the study of the interaction of intense laser light with matter. This book is a textbook on nonlinear optics at the level of a beginning graduate student. The intent of the book is to provide an introduction to the field of nonlinear optics that stresses fundamental concepts and that enables the student to go on to perform independent research in this field. This book covers the areas of nonlinear optics, quantum optics, quantum electronics, laser physics, electrooptics, and modern optics
Nonlinear light-matter interactions in engineered optical media
Litchinitser, Natalia
In this talk, we consider fundamental optical phenomena at the interface of nonlinear and singular optics in artificial media, including theoretical and experimental studies of linear and nonlinear light-matter interactions of vector and singular optical beams in metamaterials. We show that unique optical properties of metamaterials open unlimited prospects to ``engineer'' light itself. Thanks to their ability to manipulate both electric and magnetic field components, metamaterials open new degrees of freedom for tailoring complex polarization states and orbital angular momentum (OAM) of light. We will discuss several approaches to structured light manipulation on the nanoscale using metal-dielectric, all-dielectric and hyperbolic metamaterials. These new functionalities, including polarization and OAM conversion, beam magnification and de-magnification, and sub-wavelength imaging using novel non-resonant hyperlens are likely to enable a new generation of on-chip or all-fiber structured light applications. The emergence of metamaterials also has a strong potential to enable a plethora of novel nonlinear light-matter interactions and even new nonlinear materials. In particular, nonlinear focusing and defocusing effects are of paramount importance for manipulation of the minimum focusing spot size of structured light beams necessary for nanoscale trapping, manipulation, and fundamental spectroscopic studies. Colloidal suspensions offer as a promising platform for engineering polarizibilities and realization of large and tunable nonlinearities. We will present our recent studies of the phenomenon of spatial modulational instability leading to laser beam filamentation in an engineered soft-matter nonlinear medium. Finally, we introduce so-called virtual hyperbolic metamaterials formed by an array of plasma channels in air as a result of self-focusing of an intense laser pulse, and show that such structure can be used to manipulate microwave beams in a free space. This
Chen, Xianfeng; Zeng, Heping; Guo, Qi; She, Weilong
2015-01-01
This book presents an overview of the state of the art of nonlinear optics from weak light nonlinear optics, ultrafast nonlinear optics to electro-optical theory and applications. Topics range from the fundamental studies of the interaction between matter and radiation to the development of devices, components, and systems of tremendous commercial interest for widespread applications in optical telecommunications, medicine, and biotechnology.
Bloembergen, Nicolaas
1996-01-01
Nicolaas Bloembergen, recipient of the Nobel Prize for Physics (1981), wrote Nonlinear Optics in 1964, when the field of nonlinear optics was only three years old. The available literature has since grown by at least three orders of magnitude.The vitality of Nonlinear Optics is evident from the still-growing number of scientists and engineers engaged in the study of new nonlinear phenomena and in the development of new nonlinear devices in the field of opto-electronics. This monograph should be helpful in providing a historical introduction and a general background of basic ideas both for expe
Boyd, Robert W
2013-01-01
Nonlinear Optics is an advanced textbook for courses dealing with nonlinear optics, quantum electronics, laser physics, contemporary and quantum optics, and electrooptics. Its pedagogical emphasis is on fundamentals rather than particular, transitory applications. As a result, this textbook will have lasting appeal to a wide audience of electrical engineering, physics, and optics students, as well as those in related fields such as materials science and chemistry.Key Features* The origin of optical nonlinearities, including dependence on the polarization of light* A detailed treatment of the q
Nonlinear Optics and Applications
Abdeldayem, Hossin A. (Editor); Frazier, Donald O. (Editor)
2007-01-01
Nonlinear optics is the result of laser beam interaction with materials and started with the advent of lasers in the early 1960s. The field is growing daily and plays a major role in emerging photonic technology. Nonlinear optics play a major role in many of the optical applications such as optical signal processing, optical computers, ultrafast switches, ultra-short pulsed lasers, sensors, laser amplifiers, and many others. This special review volume on Nonlinear Optics and Applications is intended for those who want to be aware of the most recent technology. This book presents a survey of the recent advances of nonlinear optical applications. Emphasis will be on novel devices and materials, switching technology, optical computing, and important experimental results. Recent developments in topics which are of historical interest to researchers, and in the same time of potential use in the fields of all-optical communication and computing technologies, are also included. Additionally, a few new related topics which might provoke discussion are presented. The book includes chapters on nonlinear optics and applications; the nonlinear Schrodinger and associated equations that model spatio-temporal propagation; the supercontinuum light source; wideband ultrashort pulse fiber laser sources; lattice fabrication as well as their linear and nonlinear light guiding properties; the second-order EO effect (Pockels), the third-order (Kerr) and thermo-optical effects in optical waveguides and their applications in optical communication; and, the effect of magnetic field and its role in nonlinear optics, among other chapters.
Hanamura, Eiichi; Yamanaka, Akio
2007-01-01
This graduate-level textbook gives an introductory overview of the fundamentals of quantum nonlinear optics. Based on the quantum theory of radiation, Quantum Nonlinear Optics incorporates the exciting developments in novel nonlinear responses of materials (plus laser oscillation and superradiance) developed over the past decade. It deals with the organization of radiation field, interaction between electronic system and radiation field, statistics of light, mutual manipulation of light and matter, laser oscillation, dynamics of light, nonlinear optical response, and nonlinear spectroscopy, as well as ultrashort and ultrastrong laser pulse. Also considered are Q-switching, mode locking and pulse compression. Experimental and theoretical aspects are intertwined throughout.
Topological charge algebra of optical vortices in nonlinear interactions.
Zhdanova, Alexandra A; Shutova, Mariia; Bahari, Aysan; Zhi, Miaochan; Sokolov, Alexei V
2015-12-28
We investigate the transfer of orbital angular momentum among multiple beams involved in a coherent Raman interaction. We use a liquid crystal light modulator to shape pump and Stokes beams into optical vortices with various integer values of topological charge, and cross them in a Raman-active crystal to produce multiple Stokes and anti-Stokes sidebands. We measure the resultant vortex charges using a tilted-lens technique. We verify that in every case the generated beams' topological charges obey a simple relationship, resulting from angular momentum conservation for created and annihilated photons, or equivalently, from phase-matching considerations for multiple interacting beams.
Propagation and Interactions of Ultrahigh Power Light: Relativistic Nonlinear Optics
2014-09-30
force of the ROS causes the bucket to constantly expand, trapping copious unwanted electrons, polluting the electron spectrum with a high-charge, low...Laser Wakefield Accelerator,” Conference on Lasers and Electro-Optics/Pacific Rim , C1094, Optical Society of America (2011). 19. Bunkers, K., Kalmykov
Kuang-Leman; Wu Yong Shi
2003-01-01
We study linear and nonlinear optical properties of an electromagnetically induced transparency (EIT) medium interacting with two quantized laser fields in the adiabatic EIT case. We show that the EIT medium exhibits normal dispersion. Kerr and higher-order nonlinear refractive index coefficients are also calculated in a completely analytical form. It is indicated that the EIT medium exhibits giant resonantly enhanced nonlinearities. We discuss the response of the EIT medium to nonclassical light fields and find that the polarization vanishes when the probe laser is initially in a nonclassical state of no single-photon coherence.
Nonlinear optics at interfaces
International Nuclear Information System (INIS)
Chen, C.K.
1980-12-01
Two aspects of surface nonlinear optics are explored in this thesis. The first part is a theoretical and experimental study of nonlinear intraction of surface plasmons and bulk photons at metal-dielectric interfaces. The second part is a demonstration and study of surface enhanced second harmonic generation at rough metal surfaces. A general formulation for nonlinear interaction of surface plasmons at metal-dielectric interfaces is presented and applied to both second and third order nonlinear processes. Experimental results for coherent second and third harmonic generation by surface plasmons and surface coherent antiStokes Raman spectroscopy (CARS) are shown to be in good agreement with the theory
Leburn, Christopher; Reid, Derryck
2013-01-01
The field of ultrafast nonlinear optics is broad and multidisciplinary, and encompasses areas concerned with both the generation and measurement of ultrashort pulses of light, as well as those concerned with the applications of such pulses. Ultrashort pulses are extreme events – both in terms of their durations, and also the high peak powers which their short durations can facilitate. These extreme properties make them powerful experiment tools. On one hand, their ultrashort durations facilitate the probing and manipulation of matter on incredibly short timescales. On the other, their ultrashort durations can facilitate high peak powers which can drive highly nonlinear light-matter interaction processes. Ultrafast Nonlinear Optics covers a complete range of topics, both applied and fundamental in nature, within the area of ultrafast nonlinear optics. Chapters 1 to 4 are concerned with the generation and measurement of ultrashort pulses. Chapters 5 to 7 are concerned with fundamental applications of ultrasho...
Soto-Crespo, J M; Grelu, Philippe; Akhmediev, Nail
2006-05-01
We demonstrate the existence of stable optical light bullets in nonlinear dissipative media for both cases of normal and anomalous chromatic dispersion. The prediction is based on direct numerical simulations of the (3+1)-dimensional complex cubic-quintic Ginzburg-Landau equation. We do not impose conditions of spherical or cylindrical symmetry. Regions of existence of stable bullets are determined in the parameter space. Beyond the domain of parameters where stable bullets are found, unstable bullets can be transformed into "rockets" i.e. bullets elongated in the temporal domain. A few examples of the interaction between two optical bullets are considered using spatial and temporal interaction planes.
Quantum mechanical analysis of nonlinear optical response of interacting graphene nanoflakes
Directory of Open Access Journals (Sweden)
Hanying Deng
2018-01-01
Full Text Available We propose a distant-neighbor quantum-mechanical (DNQM approach to study the linear and nonlinear optical properties of graphene nanoflakes (GNFs. In contrast to the widely used tight-binding description of the electronic states that considers only the nearest-neighbor coupling between the atoms, our approach is more accurate and general, as it captures the electron-core interactions between all atoms in the structure. Therefore, as we demonstrate, the DNQM approach enables the investigation of the optical coupling between two closely separated but chemically unbound GNFs. We also find that the optical response of GNFs depends crucially on their shape, size, and symmetry properties. Specifically, increasing the size of nanoflakes is found to shift their accommodated quantum plasmon oscillations to lower frequency. Importantly, we show that by embedding a cavity into GNFs, one can change their symmetry properties, tune their optical properties, or enable otherwise forbidden second-harmonic generation processes.
Lugiato, Luigi; Brambilla, Massimo
2015-01-01
Guiding graduate students and researchers through the complex world of laser physics and nonlinear optics, this book provides an in-depth exploration of the dynamics of lasers and other relevant optical systems, under the umbrella of a unitary spatio-temporal vision. Adopting a balanced approach, the book covers traditional as well as special topics in laser physics, quantum electronics and nonlinear optics, treating them from the viewpoint of nonlinear dynamical systems. These include laser emission, frequency generation, solitons, optically bistable systems, pulsations and chaos and optical pattern formation. It also provides a coherent and up-to-date treatment of the hierarchy of nonlinear optical models and of the rich variety of phenomena they describe, helping readers to understand the limits of validity of each model and the connections among the phenomena. It is ideal for graduate students and researchers in nonlinear optics, quantum electronics, laser physics and photonics.
Nonlinear optics principles and applications
Li, Chunfei
2017-01-01
This book reflects the latest advances in nonlinear optics. Besides the simple, strict mathematical deduction, it also discusses the experimental verification and possible future applications, such as the all-optical switches. It consistently uses the practical unit system throughout. It employs simple physical images, such as "light waves" and "photons" to systematically explain the main principles of nonlinear optical effects. It uses the first-order nonlinear wave equation in frequency domain under the condition of “slowly varying amplitude approximation" and the classical model of the interaction between the light and electric dipole. At the same time, it also uses the rate equations based on the energy-level transition of particle systems excited by photons and the energy and momentum conservation principles to explain the nonlinear optical phenomenon. The book is intended for researchers, engineers and graduate students in the field of the optics, optoelectronics, fiber communication, information tech...
Photostable nonlinear optical polycarbonates
Faccini, M.; Balakrishnan, M.; Diemeer, Mart; Torosantucci, Riccardo; Driessen, A.; Reinhoudt, David; Verboom, Willem
2008-01-01
Highly thermal and photostable nonlinear optical polymers were obtained by covalently incorporating the tricyanovinylidenediphenylaminobenzene (TCVDPA) chromophore to a polycarbonate backbone. NLO polycarbonates with different chromophore attachment modes and flexibilities were synthesized. In spite
Nonlinear Optical Terahertz Technology
National Aeronautics and Space Administration — We develop a new approach to generation of THz radiation. Our method relies on mixing two optical frequency beams in a nonlinear crystalline Whispering Gallery Mode...
International Nuclear Information System (INIS)
Shen Yuanrang
2011-01-01
This article presents a brief introduction to the birth and early investigations of nonlinear optics, such as second harmonic generation,sum and difference frequency generation, stimulated Raman scattering,and self-action of light etc. Several important research achievements and applications of nonlinear optics are presented as well, including nonlinear optical spectroscopy, phase conjugation and adaptive optics, coherent nonlinear optics, and high-order harmonic generation. In the end, current and future research topics in nonlinear optics are summarized. (authors)
Fundamentals of nonlinear optical materials
Indian Academy of Sciences (India)
Nonlinear optics; nonlinear polarization; optical fiber communication; optical switch- ing. PACS Nos 42.65Tg; ... The importance of nonlinear optics is to understand the nonlinear behavior in the induced polarization and to ..... but much work in material development and characterization remains to be done. 16. Conclusion.
Giant nonlinear interaction between two optical beams via a quantum dot embedded in a photonic wire
Nguyen, H. A.; Grange, T.; Reznychenko, B.; Yeo, I.; de Assis, P.-L.; Tumanov, D.; Fratini, F.; Malik, N. S.; Dupuy, E.; Gregersen, N.; Auffèves, A.; Gérard, J.-M.; Claudon, J.; Poizat, J.-Ph.
2018-05-01
Optical nonlinearities usually appear for large intensities, but discrete transitions allow for giant nonlinearities operating at the single-photon level. This has been demonstrated in the last decade for a single optical mode with cold atomic gases, or single two-level systems coupled to light via a tailored photonic environment. Here, we demonstrate a two-mode giant nonlinearity with a single semiconductor quantum dot (QD) embedded in a photonic wire antenna. We exploit two detuned optical transitions associated with the exciton-biexciton QD level scheme. Owing to the broadband waveguide antenna, the two transitions are efficiently interfaced with two free-space laser beams. The reflection of one laser beam is then controlled by the other beam, with a threshold power as low as 10 photons per exciton lifetime (1.6 nW ). Such a two-color nonlinearity opens appealing perspectives for the realization of ultralow-power logical gates and optical quantum gates, and could also be implemented in an integrated photonic circuit based on planar waveguides.
Giant nonlinear interaction between two optical beams via a quantum dot embedded in a photonic wire
DEFF Research Database (Denmark)
Nguyen, H.A.; Grange, T.; Reznychenko, B.
2018-01-01
a tailored photonic environment. Here, we demonstrate a two-mode giant nonlinearity with a single semiconductor quantum dot (QD) embedded in a photonic wire antenna. We exploit two detuned optical transitions associated with the exciton-biexciton QD level scheme. Owing to the broadband waveguide antenna...
Khadzhi, P. I.; Lyakhomskaya, K. D.; Nadkin, L. Y.; Markov, D. A.
2002-05-01
The characteristic peculiarities of the self-reflection of a strong electromagnetic wave in a system of coherent excitons and biexcitons due to the exciton-photon interaction and optical exciton-biexciton conversion in semiconductors were investigated as one of the manifestations of nonlinear optical Stark-effect. It was found that a monotonously decreasing standing wave with an exponential decreasing spatial tail is formed in the semiconductor. Under the action of the field of a strong pulse, an optically homogeneous medium is converted, into the medium with distributed feedback. The appearance of the spatially separated narrow pears of the reflective index, extinction and reflection coefficients is predicted.
Nonlinear fibre optics overview
DEFF Research Database (Denmark)
Travers, J. C.; Frosz, Michael Henoch; Dudley, J. M.
2010-01-01
The optical fiber based supercontinuum source has recently become a significant scientific and commercial success, with applications ranging from frequency comb production to advanced medical imaging. This one-of-a-kind book explains the theory of fiber supercontinuum broadening, describes......, provides a background to the associated nonlinear optical processes, treats the generation mechanisms from continuous wave to femtosecond pulse pump regimes and highlights the diverse applications. A full discussion of numerical methods and comprehensive computer code are also provided, enabling readers...
Terahertz semiconductor nonlinear optics
DEFF Research Database (Denmark)
Turchinovich, Dmitry; Hvam, Jørn Märcher; Hoffmann, Matthias
2013-01-01
In this proceedings we describe our recent results on semiconductor nonlinear optics, investigated using single-cycle THz pulses. We demonstrate the nonlinear absorption and self-phase modulation of strong-field THz pulses in doped semiconductors, using n-GaAs as a model system. The THz...... nonlinearity in doped semiconductors originates from the near-instantaneous heating of free electrons in the ponderomotive potential created by electric field of the THz pulse, leading to ultrafast increase of electron effective mass by intervalley scattering. Modification of effective mass in turn leads...... to a decrease of plasma frequency in semiconductor and produces a substantial modification of THz-range material dielectric function, described by the Drude model. As a result, the nonlinearity of both absorption coefficient and refractive index of the semiconductor is observed. In particular we demonstrate...
Agrawal, Govind
2012-01-01
Since the 4e appeared, a fast evolution of the field has occurred. The 5e of this classic work provides an up-to-date account of the nonlinear phenomena occurring inside optical fibers, the basis of all our telecommunications infastructure as well as being used in the medical field. Reflecting the big developments in research, this new edition includes major new content: slow light effects, which offers a reduction in noise and power consumption and more ordered network traffic-stimulated Brillouin scattering; vectorial treatment of highly nonlinear fibers; and a brand new chapter o
DEFF Research Database (Denmark)
Parigi, V.; Bimbard, E.; Stanojevic, J.
2012-01-01
We observe and measure dispersive optical nonlinearities in an ensemble of cold Rydberg atoms placed inside an optical cavity. The experimental results are in agreement with a simple model where the optical nonlinearities are due to the progressive appearance of a Rydberg blockaded volume within...
Energy Technology Data Exchange (ETDEWEB)
Hassanabadi, Hassan, E-mail: h.hasanabadi@shahroodut.ac.ir [Physics Department, Shahrood University of Technology, P.O. Box 3619995161-316, Shahrood (Iran, Islamic Republic of); Rahimov, Hamed [Physics Department, Shahrood University of Technology, P.O. Box 3619995161-316, Shahrood (Iran, Islamic Republic of); Lu Liangliang [Department of Physics, College of Physics and Electronic Engineering, Guangzhou University, Guangzhou 510006 (China); Wang Chao [Institute of Public Administration, Guangzhou University, Guangzhou 510006 (China)
2012-05-15
In this study, a detailed investigation of the nonlinear optical properties such as optical absorption and refractive index change associated with intersubband transitions in a three-electron quantum dot in two dimensions in the presence of the Rashba spin-orbit interaction has been carried out. We present the exact wave functions and energy levels of the system. Numerical results on typical GaAs/AlGaAs materials show that the decrease of the quantum dot radius blueshifts and amplifies the absorption coefficients as well as the refractive index changes, as expected. Additionally, an increase of the optical intensity and relaxation time considerably changes the absorption coefficients and the refractive index changes. - Highlights: Black-Right-Pointing-Pointer We consider a three-electron quantum dot in 2D in the presence of the Rashba spin-orbit interaction. Black-Right-Pointing-Pointer We present the exact wave functions and energy levels of the system. Black-Right-Pointing-Pointer We apply this model for GaAs/AlGaAs materials. Black-Right-Pointing-Pointer The detailed nonlinear optical properties have been investigated.
Essentials of nonlinear optics
Murti, Y V G S
2014-01-01
Current literature on Nonlinear Optics varies widely in terms of content, style, and coverage of specific topics, relative emphasis of areas and the depth of treatment. While most of these books are excellent resources for the researchers, there is a strong need for books appropriate for presenting the subject at the undergraduate or postgraduate levels in Universities. The need for such a book to serve as a textbook at the level of the bachelors and masters courses was felt by the authors while teaching courses on nonlinear optics to students of both science and engineering during the past two decades. This book has emerged from an attempt to address the requirement of presenting the subject at college level. A one-semester course covering the essentials can effectively be designed based on this.
Mann, Nishan Singh
Photonic crystal waveguides (PCWs) are nano-scale devices offering an exciting platform for exploring and exploiting enhanced linear and nonlinear light-matter interactions, aided in-part by slowing down the group velocity (vg) of on-chip photons. However, with potential applications in telecommunications, bio-sensing and quantum computing, the road to commercialization and practical devices is hindered by our limited understanding of the influence of structural disorder on linear and nonlinear light propagation. This thesis refines and develops state-of-the-art mathematical and numerical models for understanding the important role of disorder-related optical phenomena for PCWs in the linear and optical nonlinear regime. The importance of Bloch modes is demonstrated by computing the power loss caused by disorder-induced scattering for various dispersion engineered PCWs. The theoretical results are found to be in very good agreement with related experiments and it is shown how dispersion engineered designs can minimize the Bloch fields around spatial imperfections resulting in a radical departure from the usual assumed scaling vg. -2 of backscatteringlosses. We also conduct a systematic investigation of the influence of intra-hole correlation length, a parameter characterizing disorder on backscattering losses and find the loss behaviour to be qualitatively dependent on waveguide design and frequency. We then model disorder-induced resonance shifts to compute the ensemble averaged disordered density of states, accounting for important local field effects which are crucial in achieving good qualitative agreement with experiments. Lastly, motivated by emerging experiments examining enhanced nonlinear interactions, we develop an intuitive time dependent coupled mode formalism to derive propagation equations describing nonlinear pulse propagation in the presence of disorder-induced multiple scattering. The framework establishes a natural length scale for each physical
Terahertz Nonlinear Optics in Semiconductors
DEFF Research Database (Denmark)
Turchinovich, Dmitry; Hvam, Jørn Märcher; Hoffmann, Matthias C.
2013-01-01
We demonstrate the nonlinear optical effects – selfphase modulation and saturable absorption of a single-cycle THz pulse in a semiconductor. Resulting from THz-induced modulation of Drude plasma, these nonlinear optical effects, in particular, lead to self-shortening and nonlinear spectral...... breathing of a single-cycle THz pulse in a semiconductor....
Nonlinear compression of optical solitons
Indian Academy of Sciences (India)
linear pulse propagation is the nonlinear Schrödinger (NLS) equation [1]. There are ... Optical pulse compression finds important applications in optical fibres. The pulse com ..... to thank CSIR, New Delhi for financial support in the form of SRF.
Polarization Nonlinear Optics of Quadratically Nonlinear Azopolymers
International Nuclear Information System (INIS)
Konorov, S.O.; Akimov, D.A.; Ivanov, A.A.; Petrov, A.N.; Alfimov, M.V.; Yakimanskii, A.V.; Smirnov, N.N.; Ivanova, V.N.; Kudryavtsev, V.V.; Podshivalov, A.A.; Sokolova, I.M.; Zheltikov, A.M.
2005-01-01
The polarization properties of second harmonic and sum-frequency signals generated by femtosecond laser pulses in films of polymers containing covalent groups of an azobenzothiazole chromophore polarized by an external electric field are investigated. It is shown that the methods of polarization nonlinear optics make it possible to determine the structure of oriented molecular dipoles and reveal important properties of the motion of collectivized πelectrons in organic molecules with strong optical nonlinearities. The polarization measurements show that the tensor of quadratic nonlinear optical susceptibility of chromophore fragments oriented by an external field in macromolecules of the noted azopolymers has a degenerate form. This is indicative of a predominantly one-dimensional character of motion of collectivized π electrons along an extended group of atoms in such molecules
Chirality in nonlinear optics and optical switching
Meijer, E.W.; Feringa, B.L.
1993-01-01
Chirality in molecular opto-electronics is limited sofar to the use of optically active liquid crystals and a number of optical phenomena are related to the helical macroscopic structure obtained by using one enantiomer, only. In this paper, the use of chirality in nonlinear optics and optical
Applications of nonlinear fiber optics
Agrawal, Govind
2008-01-01
* The only book describing applications of nonlinear fiber optics * Two new chapters on the latest developments: highly nonlinear fibers and quantum applications* Coverage of biomedical applications* Problems provided at the end of each chapterThe development of new highly nonlinear fibers - referred to as microstructured fibers, holey fibers and photonic crystal fibers - is the next generation technology for all-optical signal processing and biomedical applications. This new edition has been thoroughly updated to incorporate these key technology developments.The bo
Field guide to nonlinear optics
Powers, Peter E
2013-01-01
Optomechanics is a field of mechanics that addresses the specific design challenges associated with optical systems. This [i]Field Guide [/i]describes how to mount optical components, as well as how to analyze a given design. It is intended for practicing optical and mechanical engineers whose work requires knowledge in both optics and mechanics. This Field Guide is designed for those looking for a condensed and concise source of key concepts, equations, and techniques for nonlinear optics. Topics covered include technologically important effects, recent developments in nonlinear optics
Saravanan, R
2018-01-01
Non-linear optical materials have widespread and promising applications, but the efforts to understand the local structure, electron density distribution and bonding is still lacking. The present work explores the structural details, the electron density distribution and the local bond length distribution of some non-linear optical materials. It also gives estimation of the optical band gap, the particle size, crystallite size, and the elemental composition from UV-Visible analysis, SEM, XRD and EDS of some non-linear optical materials respectively.
New organic materials for optics: optical storage and nonlinear optics
International Nuclear Information System (INIS)
Gan, F.
1996-01-01
New organic materials have received considerable attention recently, due to their easy preparation and different variety. The most application fields in optics are optical storage and nonlinear optics. In optical storage the organic dyes have been used for example, in record able and erasable compact disks (CD-R, CD-E) nonlinear optical effects, such as nonlinear optical absorption, second and third order optical absorption, second and third order optical nonlinearities, can be applied for making optical limiters, optical modulators, as well as laser second and third harmonic generations. Due to high value of optical absorption and optical nonlinearity organic materials are always used as thin films in optical integration. In this paper the new experimental results have been presented, and future development has been also discussed. (author)
Nonlinear Optics: Principles and Applications
DEFF Research Database (Denmark)
Rottwitt, Karsten; Tidemand-Lichtenberg, Peter
of applications, Nonlinear Optics: Principles and Applications effectively bridges physics and mathematics with relevant applied material for real-world use. The book progresses naturally from fundamental aspects to illustrative examples, and presents a strong theoretical foundation that equips the reader...... and matter, this text focuses on the physical understanding of nonlinear optics, and explores optical material response functions in the time and frequency domain....
Distributed nonlinear optical response
DEFF Research Database (Denmark)
Nikolov, Nikola Ivanov
2005-01-01
of bound states of out of phase bright solitons and dark solitons. Also, the newly introduced analogy between the nonlocal cubic nonlinear and the quadratic nonlinear media, presented in paper B and Chapter 3 is discussed. In particular it supplies intuitive physical meaning of the formation of solitons...... in quadratic nonlinear media. In the second part of the report (Chapter 4), the possibility to obtain light with ultrabroad spectrum due to the interplay of many nonlinear effects based on cubic nonlinearity is investigated thoroughly. The contribution of stimulated Raman scattering, a delayed nonlinear...... a modified nonlinear Schroedinger model equation. Chapter 4 and papers D and E are dedicated to this part of the research....
Cascaded nonlinearities for ultrafast nonlinear optical science and applications
DEFF Research Database (Denmark)
Bache, Morten
the cascading nonlinearity is investigated in detail, especially with focus on femtosecond energetic laser pulses being subjected to this nonlinear response. Analytical, numerical and experimental results are used to understand the cascading interaction and applications are demonstrated. The defocusing soliton...... observations with analogies in fiber optics are observed numerically and experimentally, including soliton self-compression, soliton-induced resonant radiation, supercontinuum generation, optical wavebreaking and shock-front formation. All this happens despite no waveguide being present, thanks...... is of particular interest here, since it is quite unique and provides the solution to a number of standing challenges in the ultrafast nonlinear optics community. It solves the problem of catastrophic focusing and formation of a filaments in bulk glasses, which even under controlled circumstances is limited...
Extreme Nonlinear Optics An Introduction
Wegener, Martin
2005-01-01
Following the birth of the laser in 1960, the field of "nonlinear optics" rapidly emerged. Today, laser intensities and pulse durations are readily available, for which the concepts and approximations of traditional nonlinear optics no longer apply. In this regime of "extreme nonlinear optics," a large variety of novel and unusual effects arise, for example frequency doubling in inversion symmetric materials or high-harmonic generation in gases, which can lead to attosecond electromagnetic pulses or pulse trains. Other examples of "extreme nonlinear optics" cover diverse areas such as solid-state physics, atomic physics, relativistic free electrons in a vacuum and even the vacuum itself. This book starts with an introduction to the field based primarily on extensions of two famous textbook examples, namely the Lorentz oscillator model and the Drude model. Here the level of sophistication should be accessible to any undergraduate physics student. Many graphical illustrations and examples are given. The followi...
Nonlinear Optics of Hexaphenyl Nanofibers
DEFF Research Database (Denmark)
Balzer, Frank; Al-Shamery, Katharina; Neuendorf, Rolf
2003-01-01
The nonlinear optical response of films of needle-shaped para-hexaphenyl nanoaggregates on mica surfaces is investigated. Two-photon luminescence as well as optical second harmonic generation (SHG) are observed following excitation with femtosecond pulses at 770 nm. Polarization dependent...... measurements reveal that the nonlinear optical transition dipole moment is oriented with an angle of 75° with respect to the needles long axes. The absolute value of the macroscopic second-order susceptibility, averaged over a size distribution of p-6P nanoaggregates, is estimated to be of the order of 6...
Nonlinear optics an analytical approach
Mandel, Paul
2010-01-01
Based on the author's extensive teaching experience and lecture notes, this textbook provides a substantially analytical rather than descriptive presentation of nonlinear optics. Divided into five parts, with most chapters corresponding to a two-hour lecture, the book begins with a unique account of the historical development from Kirchhoff's law for the black-body radiation to Planck's quantum hypothesis and Einstein's discovery of spontaneous emission - providing all the explicit proofs. The subsequent sections deal with matter quantization, ultrashort pulse propagation in 2-level media, cavity nonlinear optics, chi(2) and chi(3) media. For graduate and PhD students in nonlinear optics or photonics, while also representing a valuable reference for researchers in these fields.
Directory of Open Access Journals (Sweden)
N. A. Veretenov
2014-09-01
and their correlation with boundaries of bistability regions has been carried out. Obtained results give the possibility to determine more rigorously the parameters region, where nonlinear effects can be observed. They can be used for development of optical logic devices and, in particular, molecular memory circuits.
Chong Li; Xiaoyong Hu; Hong Yang; Qihuang Gong
2017-01-01
We propose a scheme of unidirectional transmission in a 1D nonlinear topological photonic crystal based on the topological edge state and three order optical nonlinearity. The 1D photonic crystals consists of a nonlinear photonic crystal L and a linear photonic crystal R. In the backward direction, light is totally reflected for the photons transmission prohibited by the bandgap. While in the forward direction, light interacts with the nonlinear photonic crystal L by optical Kerr effect, brin...
Advanced in Nonlinear Optics and Laser Research and Development
International Nuclear Information System (INIS)
Jackel, S.; Kotler, Z; Lavi, R.; Sternklar, S.
1996-01-01
The Nonlinear Optics Group (NLOG) at Soreq NRC is engaged in the development of fundamental and applied technology in the related fields of nonlinear optics and laser development. Our work in nonlinear optics started with the goal of improving laser performance. These efforts were successful and opened the way for R and D in nonlinear optics for other applications. Today we use nonlinear optics to enable continuous tunability of lasers, control the path of light beams, modulate a light signal rapidly, provide optical data storage, and supply new means of microscopically probing biological and inorganic samples. Technology maturation and interaction with users will show which aspects of nonlinear optics will make the most impact
Nonlinear optics principles and applications
Rottwitt, Karsten
2014-01-01
IntroductionReview of linear opticsInduced polarizationHarmonic oscillator modelLocal field correctionsEstimated nonlinear responseSummaryTime-domain material responseThe polarization time-response functionThe Born-Oppenheimer approximationRaman scattering response function of silicaSummaryMaterial response in the frequency domain, susceptibility tensorsThe susceptibility tensorThe induced polarization in the frequency domainSum of monochromatic fieldsThe prefactor to the induced polarizationThird-order polarization in the Born-Oppenheimer approximation in the frequency domainKramers-Kronig relationsSummarySymmetries in nonlinear opticsSpatial symmetriesSecond-order materialsThird-order nonlinear materialsCyclic coordinate-systemContracted notation for second-order susceptibility tensorsSummaryThe nonlinear wave equationMono and quasi-monochromatic beamsPlane waves - the transverse problemWaveguidesVectorial approachNonlinear birefringenceSummarySecond-order nonlinear effectsGeneral theoryCoupled wave theoryP...
Oscillating solitons in nonlinear optics
Indian Academy of Sciences (India)
... are derived, and the relevant properties and features of oscillating solitons are illustrated. Oscillating solitons are controlled by the reciprocal of the group velocity and Kerr nonlinearity. Results of this paper will be valuable to the study of dispersion-managed optical communication system and mode-locked fibre lasers.
Nonlinear optical properties of silicon waveguides
International Nuclear Information System (INIS)
Tsang, H K; Liu, Y
2008-01-01
Recent work on two-photon absorption (TPA), stimulated Raman scattering (SRS) and optical Kerr effect in silicon-on-insulator (SOI) waveguides is reviewed and some potential applications of these optical nonlinearities, including silicon-based autocorrelation detectors, optical amplifiers, high speed optical switches, optical wavelength converters and self-phase modulation (SPM), are highlighted. The importance of free carriers generated by TPA in nonlinear devices is discussed, and a generalized definition of the nonlinear effective length to cater for nonlinear losses is proposed. How carrier lifetime engineering, and in particular the use of helium ion implantation, can enhance the nonlinear effective length for nonlinear devices is also discussed
Nonlinear fiber optics formerly quantum electronics
Agrawal, Govind
1995-01-01
The field of nonlinear fiber optics has grown substantially since the First Edition of Nonlinear Fiber Optics, published in 1989. Like the First Edition, this Second Edition is a comprehensive, tutorial, and up-to-date account of nonlinear optical phenomena in fiber optics. It synthesizes widely scattered research material and presents it in an accessible manner for students and researchers already engaged in or wishing to enter the field of nonlinear fiber optics. Particular attention is paid to the importance of nonlinear effects in the design of optical fiber communication systems. This is
Rigorous theory of molecular orientational nonlinear optics
International Nuclear Information System (INIS)
Kwak, Chong Hoon; Kim, Gun Yeup
2015-01-01
Classical statistical mechanics of the molecular optics theory proposed by Buckingham [A. D. Buckingham and J. A. Pople, Proc. Phys. Soc. A 68, 905 (1955)] has been extended to describe the field induced molecular orientational polarization effects on nonlinear optics. In this paper, we present the generalized molecular orientational nonlinear optical processes (MONLO) through the calculation of the classical orientational averaging using the Boltzmann type time-averaged orientational interaction energy in the randomly oriented molecular system under the influence of applied electric fields. The focal points of the calculation are (1) the derivation of rigorous tensorial components of the effective molecular hyperpolarizabilities, (2) the molecular orientational polarizations and the electronic polarizations including the well-known third-order dc polarization, dc electric field induced Kerr effect (dc Kerr effect), optical Kerr effect (OKE), dc electric field induced second harmonic generation (EFISH), degenerate four wave mixing (DFWM) and third harmonic generation (THG). We also present some of the new predictive MONLO processes. For second-order MONLO, second-order optical rectification (SOR), Pockels effect and difference frequency generation (DFG) are described in terms of the anisotropic coefficients of first hyperpolarizability. And, for third-order MONLO, third-order optical rectification (TOR), dc electric field induced difference frequency generation (EFIDFG) and pump-probe transmission are presented
Nonlinear optical crystals a complete survey
Nikogosyan, David N
2005-01-01
Nonlinear optical crystals are widely used in modern optical science and technology for frequency conversion of laser light, i.e. to generate laser radiation at any specific wavelength in visible, UV or IR spectral regions. This unrivalled reference book contains the most complete and up-to-date information on properties of nonlinear optical crystals. It includes: * Database of 63 common and novel nonlinear optical crystals * Periodically-poled and self-frequency-doubling materials * Full description of linear and nonlinear optical properties * Significant amount of crystallophysical, thermophysical, spectroscopic, electro-optic and magneto-optic information * 7 mini-reviews on novel applications, such as deep-UV light generation, terahertz-wave generation, ultrashort laser pulse compression, photonic band-gap crystals, x3 nonlinearity, etc. * More than 1500 different references with full titles It is a vital source of information for scientists and engineers dealing with modern applications of nonlinear opti...
Nonlinear optical studies of surfaces
International Nuclear Information System (INIS)
Shen, Y.R.
1994-07-01
The possibly of using nonlinear optical processes for surface studies has attracted increasing attention in recent years. Optical second harmonic generation (SHG) and sum frequency generation (SFG), in particular, have been well accepted as viable surface probes. They have many advantages over the conventional techniques. By nature, they are highly surface-specific and has a submonolayer sensitivity. As coherent optical processes, they are capable of in-situ probing of surfaces in hostile environment as well as applicable to all interfaces accessible by light. With ultrafast pump laser pulses, they can be employed to study surface dynamic processes with a subpicosecond time resolution. These advantages have opened the door to many exciting research opportunities in surface science and technology. This paper gives a brief overview of this fast-growing new area of research. Optical SHG from a surface was first studied theoretically and experimentally in the sixties. Even the submonolayer surface sensitivity of the process was noticed fairly early. The success was, however, limited because of difficulties in controlling the experimental conditions. It was not until the early 1980's that the potential of the process for surface analysis was duly recognized. The first surface study by SHG was actually motivated by the then active search for an understanding of the intriguing surface enhanced Raman scattering (SERS). It had been suspected that the enhancement in SERS mainly came from the local-field enhancement due to local plasmon resonances and pointing rod effect on rough metal surfaces. In our view, Raman scattering is a two-photon process and is therefore a nonlinear optical effect
Nonlinear Optical Fiber Arrays for Limiting Application
National Research Council Canada - National Science Library
Khoo, Iam-Choon
2006-01-01
.... Measurements show that they possess desirable nonlinear optical such as low-freezing pint, non-volatile, transparent for low light level and possess large effective nonlinear absorption coefficients...
Nanoplasmonic solution for nonlinear optics
DEFF Research Database (Denmark)
Bache, Morten; Lavrinenko, Andrei; Lysenko, Oleg
2014-01-01
for the silicon dioxide cladding. The blue, cyan and magenta curves correspond to the transmission spectra for the gold waveguides with the width of 10 μm and length of 2, 3, and 4 mm.The polarization of laser beam was tuned to match the transverse magnetic mode of surface plasmonpolaritons in the gold waveguides...... and is being under investigation in recent years [3].The purpose of our research is to study nonlinear optical properties of gold waveguides embedded intodielectric medium (silicon dioxide) using picosecond laser spectroscopy. The work includes modeling ofoptical properties of gold waveguides, fabrication...... of prototype samples, and optical characterization ofsamples using a picosecond laser source.The prototype samples of gold waveguides embedded into silicon dioxide were fabricated at DTUDanchip. A silicon wafer with pre-made 6.5 μm layer of silicon dioxide was used as a substrate and goldwaveguides (films...
Nonlinear Photonics and Novel Optical Phenomena
Morandotti, Roberto
2012-01-01
Nonlinear Photonics and Novel Optical Phenomena contains contributed chapters from leading experts in nonlinear optics and photonics, and provides a comprehensive survey of fundamental concepts as well as hot topics in current research on nonlinear optical waves and related novel phenomena. The book covers self-accelerating airy beams, integrated photonics based on high index doped-silica glass, linear and nonlinear spatial beam dynamics in photonic lattices and waveguide arrays, polariton solitons and localized structures in semiconductor microcavities, terahertz waves, and other novel phenomena in different nanophotonic and optical systems.
Biological applications of novel nonlinear optical microscopy
International Nuclear Information System (INIS)
Kajiyama, Shin'ichiro; Ozeki, Yasuyuki; Itoh, Kazuyoshi; Fukui, Kiichi
2010-01-01
Two types of newly developed nonlinear optical microscopes namely stimulated parametric emission (SPE) microscope and stimulated Raman scattering (SRS) microscope were presented together with their biological applications.
Cavity nonlinear optics with layered materials
Directory of Open Access Journals (Sweden)
Fryett Taylor
2017-12-01
Full Text Available Unprecedented material compatibility and ease of integration, in addition to the unique and diverse optoelectronic properties of layered materials, have generated significant interest in their utilization in nanophotonic devices. While initial nanophotonic experiments with layered materials primarily focused on light sources, modulators, and detectors, recent efforts have included nonlinear optical devices. In this paper, we review the current state of cavity-enhanced nonlinear optics with layered materials. Along with conventional nonlinear optics related to harmonic generation, we report on emerging directions of nonlinear optics, where layered materials can potentially play a significant role.
Nonlinear optics of fibre event horizons.
Webb, Karen E; Erkintalo, Miro; Xu, Yiqing; Broderick, Neil G R; Dudley, John M; Genty, Goëry; Murdoch, Stuart G
2014-09-17
The nonlinear interaction of light in an optical fibre can mimic the physics at an event horizon. This analogue arises when a weak probe wave is unable to pass through an intense soliton, despite propagating at a different velocity. To date, these dynamics have been described in the time domain in terms of a soliton-induced refractive index barrier that modifies the velocity of the probe. Here we complete the physical description of fibre-optic event horizons by presenting a full frequency-domain description in terms of cascaded four-wave mixing between discrete single-frequency fields, and experimentally demonstrate signature frequency shifts using continuous wave lasers. Our description is confirmed by the remarkable agreement with experiments performed in the continuum limit, reached using ultrafast lasers. We anticipate that clarifying the description of fibre event horizons will significantly impact on the description of horizon dynamics and soliton interactions in photonics and other systems.
Progress in nonlinear nano-optics
Lienau, Christoph; Grunwald, Rüdiger
2015-01-01
This book presents the state of the art in nonlinear nanostructures for ultrafast laser applications. Most recent results in two emerging fields are presented: (i) generation of laser-induced nanostructures in materials like metals, metal oxides and semiconductors, and (ii) ultrafast excitation and energy transfer in nanoscale physical, chemical and hybrid systems. Particular emphasis is laid on the up-to-date controversially discussed mechanisms of sub-wavelength ripple formation including models of self-organized material transport and multiphoton excitation channels, nonlinear optics of plasmonic structures (nanotips, nanowires, 3D-metamaterials), and energy localization and transport on ultrafast time scale and spatial nanoscale. High-resolution spectroscopy, simulation and characterization techniques are reported. New applications of ultrashort-pulsed lasers for materials processing and the use of nanostructured materials for characterizing laser fields and laser-matter-interactions are discussed.
Nonlinear and quantum optics near nanoparticles
Dhayal, Suman
We study the behavior of electric fields in and around dielectric and metal nanoparticles, and prepare the ground for their applications to a variety of systems viz. photovoltaics, imaging and detection techniques, and molecular spectroscopy. We exploit the property of nanoparticles being able to focus the radiation field into small regions and study some of the interesting nonlinear, and quantum coherence and interference phenomena near them. The traditional approach to study the nonlinear light-matter interactions involves the use of the slowly varying amplitude approximation (SVAA) as it simplifies the theoretical analysis. However, SVVA cannot be used for systems which are of the order of the wavelength of the light. We use the exact solutions of the Maxwell's equations to obtain the fields created due to metal and dielectric nanoparticles, and study nonlinear and quantum optical phenomena near these nanoparticles. We begin with the theoretical description of the electromagnetic fields created due to the nonlinear wavemixing process, namely, second-order nonlinearity in an nonlinear sphere. The phase-matching condition has been revisited in such particles and we found that it is not satisfied in the sphere. We have suggested a way to obtain optimal conditions for any type and size of material medium. We have also studied the modifications of the electromagnetic fields in a collection of nanoparticles due to strong near field nonlinear interactions using the generalized Mie theory for the case of many particles applicable in photovoltaics (PV). We also consider quantum coherence phenomena such as modification of dark states, stimulated Raman adiabatic passage (STIRAP), optical pumping in 4-level atoms near nanoparticles by using rotating wave approximation to describe the Hamiltonian of the atomic system. We also considered the behavior of atomic and the averaged atomic polarization in 7-level atoms near nanoparticles. This could be used as a prototype to study
Nonlinear optics quantum computing with circuit QED.
Adhikari, Prabin; Hafezi, Mohammad; Taylor, J M
2013-02-08
One approach to quantum information processing is to use photons as quantum bits and rely on linear optical elements for most operations. However, some optical nonlinearity is necessary to enable universal quantum computing. Here, we suggest a circuit-QED approach to nonlinear optics quantum computing in the microwave regime, including a deterministic two-photon phase gate. Our specific example uses a hybrid quantum system comprising a LC resonator coupled to a superconducting flux qubit to implement a nonlinear coupling. Compared to the self-Kerr nonlinearity, we find that our approach has improved tolerance to noise in the qubit while maintaining fast operation.
Interactive Nonlinear Multiobjective Optimization Methods
Miettinen, Kaisa; Hakanen, Jussi; Podkopaev, Dmitry
2016-01-01
An overview of interactive methods for solving nonlinear multiobjective optimization problems is given. In interactive methods, the decision maker progressively provides preference information so that the most satisfactory Pareto optimal solution can be found for her or his. The basic features of several methods are introduced and some theoretical results are provided. In addition, references to modifications and applications as well as to other methods are indicated. As the...
Nonlinear optics of liquid crystalline materials
International Nuclear Information System (INIS)
Khoo, Iam Choon
2009-01-01
Liquid crystals occupy an important niche in nonlinear optics as a result of their unique physical and optical properties. Besides their broadband birefringence and transparency, abilities to self-assemble into various crystalline phases and to conform to various flexible forms and shapes, liquid crystals are compatible with almost all other optoelectronic materials and technology platforms. In both isotropic and ordered phases, liquid crystals possess extraordinarily large optical nonlinearities that stretch over multiple time scales. To date, almost all conceivable nonlinear optical phenomena have been observed in a very broad spectrum spanning the entire visible to infrared and beyond. In this review, we present a self-contained complete discussion of the optical nonlinearities of liquid crystals, and a thorough review of a wide range of nonlinear optical processes and phenomena enabled by these unique properties. Starting with a brief historical account of the development of nonlinear optical studies of the mesophases of liquid crystals, we then review various liquid crystalline materials and structures, and their nonlinear optical properties. Emphasis is placed on the nematic phase, which best exemplifies the dual nature of liquid crystals, although frequent references to other phases are also made. We also delve into recent work on novel structures such as photonic crystals, metamaterials and nanostructures and their special characteristics and emergent properties. The mechanisms and complex nonlocal dynamics of optical nonlinearities associated with laser induced director axis reorientation, thermal, density, and order parameter fluctuations, space charge field formation and photorefractivity are critically reviewed as a foundation for the discussions of various nonlinear optical processes detailed in this paper
Optical Chirality in Nonlinear Optics: Application to High Harmonic Generation.
Neufeld, Ofer; Cohen, Oren
2018-03-30
Optical chirality (OC)-one of the fundamental quantities of electromagnetic fields-corresponds to the instantaneous chirality of light. It has been utilized for exploring chiral light-matter interactions in linear optics, but has not yet been applied to nonlinear processes. Motivated to explore the role of OC in the generation of helically polarized high-order harmonics and attosecond pulses, we first separate the OC of transversal and paraxial beams to polarization and orbital terms. We find that the polarization-associated OC of attosecond pulses corresponds approximately to that of the pump in the quasimonochromatic case, but not in the multichromatic pump cases. We associate this discrepancy with the fact that the polarization OC of multichromatic pumps vary rapidly in time along the optical cycle. Thus, we propose new quantities, noninstantaneous polarization-associated OC, and time-scale-weighted polarization-associated OC, and show that these quantities link the chirality of multichromatic pumps and their generated attosecond pulses. The presented extension to OC theory should be useful for exploring various nonlinear chiral light-matter interactions. For example, it stimulates us to propose a tricircular pump for generation of highly elliptical attosecond pulses with a tunable ellipticity.
Optical Chirality in Nonlinear Optics: Application to High Harmonic Generation
Neufeld, Ofer; Cohen, Oren
2018-03-01
Optical chirality (OC)—one of the fundamental quantities of electromagnetic fields—corresponds to the instantaneous chirality of light. It has been utilized for exploring chiral light-matter interactions in linear optics, but has not yet been applied to nonlinear processes. Motivated to explore the role of OC in the generation of helically polarized high-order harmonics and attosecond pulses, we first separate the OC of transversal and paraxial beams to polarization and orbital terms. We find that the polarization-associated OC of attosecond pulses corresponds approximately to that of the pump in the quasimonochromatic case, but not in the multichromatic pump cases. We associate this discrepancy with the fact that the polarization OC of multichromatic pumps vary rapidly in time along the optical cycle. Thus, we propose new quantities, noninstantaneous polarization-associated OC, and time-scale-weighted polarization-associated OC, and show that these quantities link the chirality of multichromatic pumps and their generated attosecond pulses. The presented extension to OC theory should be useful for exploring various nonlinear chiral light-matter interactions. For example, it stimulates us to propose a tricircular pump for generation of highly elliptical attosecond pulses with a tunable ellipticity.
International Nuclear Information System (INIS)
Lalousis, P.
1984-01-01
Nonthermal direct electrodynamic interaction between laser energy and a fully ionized plasma was studied. The particular emphasis is on the action of nonlinear forces, in which the optical electromagnetic fields act on the plasma electrons which then transfer their energy to the ions electrostatically. Instead of the usual single fluid model, the plasma is treated as two separate conducting fluids for electrons and ions, coupled by momentum and Coulomb interactions. The equations governing the two fluids are derived from first principles, and numerical algorithms for computing these equations are developed, enabling the plasma oscillatons to be resolved and studied. Fully ionized plasma expansion without laser irradiation is studied first numerically. Remarkable damping mechanisms by coupling to ion oscillations have been observed. Inhomogeneities in densities of the two fluids result in large electrostatic fields and double layers are generated. There is quite close agreement between numerically calculated electrostatic fields and analytical solutions. Laser interaction with fully ionized plasma is also studied numerically. The generation of cavitons is numerically observed, and it is inferred that laser plasma interactions produce very high electrostatic fields in the vicinity of cavitons. It is further shown that charge neutrality is not necessarily maintained in a caviton
Nonlinear laser-plasma interactions
Kaw, P. K.
2017-12-01
Soon after lasers were invented, there was tremendous curiosity on the nonlinear phenomena which would result in their interaction with a fully ionized plasma. Apart from the basic interest, it was realized that it could be used for the achievement of nuclear fusion in the laboratory. This led us to a paper on the propagation of a laser beam into an inhomogeneous fusion plasma, where it was first demonstrated that light would go up to the critical layer (where the frequency matches the plasma frequency) and get reflected from there with a reflection coefficient of order unity. The reflection coefficient was determined by collisional effects. Since the wave was expected to slow down to near zero group speed at the reflection point, the dominant collision frequency determining the reflection coefficient was the collision frequency at the reflection point. It turned out that the absorption of light was rather small for fusion temperatures. This placed a premium on investigation of nonlinear phenomena which might contribute to the absorption and penetration of the light into high-density plasma. An early investigation showed that electron jitter with respect to ions would be responsible for the excitation of decay instabilities which convert light waves into electrostatic plasma waves and ion waves near the critical frequency. These electrostatic waves would then get absorbed into the plasma even in the collisionless case and lead to plasma heating which is nonlinear. Detailed estimates of this heating were made. Similar nonlinear processes which could lead to stimulated scattering of light in the underdense region (ω >ω _p) were investigated together with a number of other workers. All these nonlinear processes need a critical threshold power for excitation. Another important process which was discovered around the same time had to do with filamentation and trapping of light when certain thresholds were exceeded. All of this work has been extensively verified in
Nonlinear soliton matching between optical fibers
DEFF Research Database (Denmark)
Agger, Christian; Sørensen, Simon Toft; Thomsen, Carsten L.
2011-01-01
In this Letter, we propose a generic nonlinear coupling coefficient, η2 NL ¼ ηjγ=β2jfiber2=jγ=β2jfiber1, which gives a quantitative measure for the efficiency of nonlinear matching of optical fibers by describing how a fundamental soliton couples from one fiber into another. Specifically, we use η...
Nuclear matter as a nonlinear optical medium
International Nuclear Information System (INIS)
Hefter, E.F.; Papini, G.
1986-01-01
This paper is concerned with the question whether nuclear matter should be considered as a nonlinear optical medium. Taking, in a pragmatic way, quality and quantity of the results of well-established linear and nonlinear approaches as the main criterion, an affirmative answer is seen to be consistent with long-standing practices adhered to in nuclear physics
Microresonators for Nonlinear Quantum Optics
Vernon, Zachary
In this thesis I study in detail the quantum dynamics of several nonlinear optical processes in microresonator systems. A Heisenberg-picture input-output formalism is developed from first principles that includes the effects of scattering losses and independent quality factors and coupling ratios for different resonances. The task of calculating the device output is then reduced to solving a set of driven, damped, ordinary differential equations for the resonator mode operators alone. This theoretical framework is used to study photon pair generation via spontaneous four-wave mixing in the weakly pumped regime, on which the effects of scattering losses are appraised. A more strongly driven regime is studied for continuous wave pumps, demonstrating when self- and cross-phase modulation and multi-photon pair generation become important, and their effects on the spectral and power scaling properties of the system are examined; A detuning strategy is presented that compensates for some of these effects. The results of the weak-pump regime are applied to study microresonator-based heralded single photon sources. The impact of scattering losses is studied, revealing that typical systems suffer from low heralding efficiency due to these losses. A technique to improve heralding efficiency is presented through over-coupling the resonator-channel system, and a resultant trade-off between heralding rate and heralding efficiency is uncovered. Limitations to the spectral purity of the heralded single photon output for conventional microresonator systems are also analysed, and a more sophisticated coupling scheme presented to overcome the upper bound for spectral purity of 93% that exists in typical systems, permitting the generation of single photons with spectral purity arbitrarily close to 100% without spectral filtering or sophisticated phase-matching techniques. The theory of quantum frequency conversion in microresonators using four-wave mixing is then developed in detail
Black phosphorus: broadband nonlinear optical absorption and application
Li, Ying; He, Yanliang; Cai, Yao; Chen, Shuqing; Liu, Jun; Chen, Yu; Yuanjiang, Xiang
2018-02-01
Black phosphorus (BP), 2D layered material with layered dependent direct bandgap (0.3 eV (bulk), 2.0 eV (single layer)) that has gained renewed attention, has been demonstrated as an extremely appropriate optical material for broadband optical applications from infrared to mid-infrared wavebands. Herein, by coupling multi-layer BP films with microfiber, we fabricated a nonlinear optical device with long light-matter interaction distance and enhanced damage threshold. Through taking full advantage of its fine nonlinear optical absorption property, we obtained stable mode-locking (51 ps) and Q-switched mode-locking states in Yb-doped or Er-doped (403.7 fs) all-fiber lasers and the single-longitudinal-mode operation (53 kHz) in an Er-doped fiber laser with enhanced power tolerance, using the same nonlinear optical device. Our results showed that BP could be a favorable nonlinear optical material for developing BP-enabled wave-guiding photonic devices, and revealed new insight into BP for high optical power unexplored optical devices.
Nonlinear optical model for strip plasmonic waveguides
DEFF Research Database (Denmark)
Lysenko, Oleg; Bache, Morten; Lavrinenko, Andrei
2016-01-01
This paper presents a theoretical model of nonlinear optical properties for strip plasmonic waveguides. The particular waveguides geometry that we investigate contains a gold core, adhesion layers, and silicon dioxide cladding. It is shown that the third-order susceptibility of the gold core...... significantly depends on the layer thickness and has the dominant contribution to the effective third-order susceptibility of the long-range plasmon polariton mode. This results in two nonlinear optical effects in plasmonic waveguides, which we experimentally observed and reported in [Opt. Lett. 41, 317 (2016...... approaches. (C) 2016 Optical Society of America...
Optical rogue waves and soliton turbulence in nonlinear fibre optics
DEFF Research Database (Denmark)
Genty, G.; Dudley, J. M.; de Sterke, C. M.
2009-01-01
We examine optical rogue wave generation in nonlinear fibre propagation in terms of soliton turbulence. We show that higher-order dispersion is sufficient to generate localized rogue soliton structures, and Raman scattering effects are not required.......We examine optical rogue wave generation in nonlinear fibre propagation in terms of soliton turbulence. We show that higher-order dispersion is sufficient to generate localized rogue soliton structures, and Raman scattering effects are not required....
International Nuclear Information System (INIS)
Zhang Rui; Garner, Sean R.; Hau, Lene Vestergaard
2009-01-01
A Bose-Einstein condensate confined in an optical dipole trap is used to generate long-term coherent memory for light, and storage times of more than 1 s are observed. Phase coherence of the condensate as well as controlled manipulations of elastic and inelastic atomic scattering processes are utilized to increase the storage fidelity by several orders of magnitude over previous schemes. The results have important applications for creation of long-distance quantum networks and for generation of entangled states of light and matter.
Nonlinear and quantum optics with liquid crystals
International Nuclear Information System (INIS)
Lukishova, Svetlana G
2014-01-01
Thermotropic liquid crystals' usual application is display technology. This paper describes experiments on light interaction with pure and doped liquid crystals under for these materials unconventional incident light powers: (1) under high-power laser irradiation, and (2) at the single-photon level. In (1), I will outline several nonlinear optical effects under high-power, nanosecond laser irradiation which should be taken into account in the design of lasers with liquid crystal components and in fabrication of optical power limiters based on liquid crystals: (1.1) athermal helical pitch dilation and unwinding of cholesteric mirrors (both in free space and inside laser resonators); (1.2) some pitfalls in measurements of refractive nonlinearity using z-scan technique under two-photon or linear absorption of liquids; (1.3) the first observation of thermal lens effects in liquid crystals under several-nanosecond, low-pulse-repetition rate (2-10 Hz) laser irradiation in the presence of two-photon absorption; (1.4) feedback-free kaleidoscope of patterns (hexagons, stripes, etc.) in dye-doped liquid crystals. In (2), at the single-photon level, it will be shown that with a proper selection of liquid crystals and a single-emitter dopant spectral range, liquid crystal structures can be used to control emitted single photons (both polarization and count rate). The application of the latter research is absolutely secure quantum communication with polarization coding of information. In particular, in (2.1), definite handedness, circular polarized cholesteric microcavity resonance in quantum dot fluorescence is reported. In (2.2), definite linear polarization of single (antibunched) photons from single-dye-molecules in planar-aligned nematic host is discussed. In (2.3), some results on photon antibunching from NV-color center in nanodiamond in liquid crystal host and circularly polarized fluorescence of definite handedness from nanocrystals doped with trivalent ions of
Oscillating solitons in nonlinear optics
Indian Academy of Sciences (India)
The study of solitons in those physical systems reveals some exciting .... With the following power series expansions for g(z,t) and f(z,t): g(z,t) = εg1(z,t) + ... If nonlinearity γ (z) is also taken as a function in figure 1b, the periodic and oscillation.
Directory of Open Access Journals (Sweden)
Chong Li
2017-02-01
Full Text Available We propose a scheme of unidirectional transmission in a 1D nonlinear topological photonic crystal based on the topological edge state and three order optical nonlinearity. The 1D photonic crystals consists of a nonlinear photonic crystal L and a linear photonic crystal R. In the backward direction, light is totally reflected for the photons transmission prohibited by the bandgap. While in the forward direction, light interacts with the nonlinear photonic crystal L by optical Kerr effect, bringing a topological phase reversal and results the topological edge mode arising at the interface which could transmit photons through the bandgaps both of the photonic crystal L and R. When the signal power intensity larger than a moderate low threshold value of 10.0 MW/cm2, the transmission contrast ratio could remain at 30 steadily.
Nonlinear optical techniques for surface studies
International Nuclear Information System (INIS)
Shen, Y.R.
1981-09-01
Recent effort in developing nonlinear optical techniques for surface studies is reviewed. Emphasis is on monolayer detection of adsorbed molecules on surfaces. It is shown that surface coherent antiStokes Raman scattering (CARS) with picosecond pulses has the sensitivity of detecting submonolayer of molecules. On the other hand, second harmonic or sum-frequency generation is also sensitive enough to detect molecular monolayers. Surface-enhanced nonlinear optical effects on some rough metal surfaces have been observed. This facilitates the detection of molecular monolayers on such surfaces, and makes the study of molecular adsorption at a liquid-metal interface feasible. Advantages and disadvantages of the nonlinear optical techniques for surface studies are discussed
Nonlinear Optics with 2D Layered Materials.
Autere, Anton; Jussila, Henri; Dai, Yunyun; Wang, Yadong; Lipsanen, Harri; Sun, Zhipei
2018-03-25
2D layered materials (2DLMs) are a subject of intense research for a wide variety of applications (e.g., electronics, photonics, and optoelectronics) due to their unique physical properties. Most recently, increasing research efforts on 2DLMs are projected toward the nonlinear optical properties of 2DLMs, which are not only fascinating from the fundamental science point of view but also intriguing for various potential applications. Here, the current state of the art in the field of nonlinear optics based on 2DLMs and their hybrid structures (e.g., mixed-dimensional heterostructures, plasmonic structures, and silicon/fiber integrated structures) is reviewed. Several potential perspectives and possible future research directions of these promising nanomaterials for nonlinear optics are also presented. © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Demkin, Artem S.; Nikitin, Dmitriy G.; Ryabushkin, Oleg A.
2016-04-01
In current work optical properties of LiB3O5 (LBO) crystal with ultraviolet (UV) (λ= 266 nm) induced volume macroscopic defect (track) are investigated using novel piezoelectric resonance laser calorimetry technique. Pulsed laser radiation of 10 W average power at 532 nm wavelength, is consecutively focused into spatial regions with and without optical defect. For these cases exponential fitting of crystal temperature kinetics measured during its irradiation gives different optical absorption coefficients α1 = 8.1 • 10-4 cm-1 (region with defect) and α =3.9ṡ10-4 cm-1 (non-defected region). Optical scattering coefficient is determined as the difference between optical absorption coefficients measured for opaque and transparent lateral facets of the crystal respectively. Measurements reveal that scattering coefficient of LBO in the region with defect is three times higher than the optical absorption coefficient.
Interactive virtual optical laboratories
Liu, Xuan; Yang, Yi
2017-08-01
Laboratory experiences are essential for optics education. However, college students have limited access to advanced optical equipment that is generally expensive and complicated. Hence there is a need for innovative solutions to expose students to advanced optics laboratories. Here we describe a novel approach, interactive virtual optical laboratory (IVOL) that allows unlimited number of students to participate the lab session remotely through internet, to improve laboratory education in photonics. Although students are not physically conducting the experiment, IVOL is designed to engage students, by actively involving students in the decision making process throughout the experiment.
Measurement-induced nonlinearity in linear optics
International Nuclear Information System (INIS)
Scheel, Stefan; Knight, Peter L.; Nemoto, Kae; Munro, William J.
2003-01-01
We investigate the generation of nonlinear operators with single-photon sources, linear optical elements, and appropriate measurements of auxiliary modes. We provide a framework for the construction of useful single-mode and two-mode quantum gates necessary for all-optical quantum information processing. We focus our attention generally on using minimal physical resources while providing a transparent and algorithmic way of constructing these operators
Nonlinear microstructured polymer optical fibres
DEFF Research Database (Denmark)
Frosz, Michael Henoch
is potentially the case for microstructured polymer optical fibres (mPOFs). Another advantage is that polymer materials have a higher biocompatibility than silica, meaning that it is easier to bond certain types of biosensor materials to a polymer surface than to silica. As with silica PCFs, it is difficult...
Anisotropic and nonlinear optical waveguides
Someda, CG
1992-01-01
Dielectric optical waveguides have been investigated for more than two decades. In the last ten years they have had the unique position of being simultaneously the backbone of a very practical and fully developed technology, as well as an extremely exciting area of basic, forefront research. Existing waveguides can be divided into two sets: one consisting of waveguides which are already in practical use, and the second of those which are still at the laboratory stage of their evolution. This book is divided into two separate parts: the first dealing with anisotropic waveguides, an
Quantum Information Processing using Nonlinear Optical Effects
DEFF Research Database (Denmark)
Andersen, Lasse Mejling
This PhD thesis treats applications of nonlinear optical effects for quantum information processing. The two main applications are four-wave mixing in the form of Bragg scattering (BS) for quantum-state-preserving frequency conversion, and sum-frequency generation (SFG) in second-order nonlinear......-chirping the pumps. In the high-conversion regime without the effects of NPM, exact Green functions for BS are derived. In this limit, separability is possible for conversion efficiencies up to 60 %. However, the system still allows for selective frequency conversion as well as re-shaping of the output. One way...
Laser beam propagation in nonlinear optical media
Guha, Shekhar
2013-01-01
""This is very unique and promises to be an extremely useful guide to a host of workers in the field. They have given a generalized presentation likely to cover most if not all situations to be encountered in the laboratory, yet also highlight several specific examples that clearly illustrate the methods. They have provided an admirable contribution to the community. If someone makes their living by designing lasers, optical parametric oscillators or other devices employing nonlinear crystals, or designing experiments incorporating laser beam propagation through linear or nonlinear media, then
Order and chaos in polarized nonlinear optics
International Nuclear Information System (INIS)
Holm, D.D.
1990-01-01
Methods for investigating temporal complexity in Hamiltonian systems are applied to the dynamics of a polarized optical laser beam propagating as a travelling wave in a medium with cubically nonlinear polarizability (i.e., a Kerr medium). The theory of Hamiltonian systems with symmetry is used to study the geometry of phase space for the optical problem, transforming from C 2 to S 2 x (J,θ), where (J,θ) is a symplectic action-angle pair. The bifurcations of the phase portraits of the Hamiltonian motion on S 2 are classified and shown graphically. These bifurcations create various saddle connections on S 2 as either J (the beam intensity), or the optical parameters of the medium are varied. After this bifurcation analysis, the Melnikov method is used to demonstrate analytically that the saddle connections break and intersect transversely in a Poincare map under spatially periodic perturbations of the optical parameters of the medium. These transverse intersections in the Poincare map imply intermittent polarization switching with extreme sensitivity to initial conditions characterized by a Smale horseshoe construction for the travelling waves of a polarized optical laser pulse. The resulting chaotic behavior in the form of sensitive dependence on initial conditions may have implications for the control and predictability of nonlinear optical polarization switching in birefringent media. 19 refs., 2 figs., 1 tab
Nonlinear ultrafast optical response in organic molecular crystals
Rahman, Talat S.; Turkowski, Volodymyr; Leuenberger, Michael N.
2012-02-01
We analyze possible nonlinear excitonic effects in the organic molecule crystals by using a combined time-dependent DFT and many-body approach. In particular, we analyze possible effects of the time-dependent (retarded)interaction between different types of excitations, Frenkel excitons, charge transfer excitons and excimers, on the electric and the optical response of the system. We pay special attention to the case of constant electric field and ultrafast pulses, including that of four-wave mixing experiments. As a specific application we examine the optical excitations of pentacene nanocrystals and compare the results with available experimental data.[1] Our results demostrate that the nonlinear effects can play an important role in the optical response of these systems. [1] A. Kabakchiev, ``Scanning Tunneling Luminescence of Pentacene Nanocrystals'', PhD Thesis (EPFL, Lausanne, 2010).
Second-order nonlinear optical microscopy of spider silk
Zhao, Yue; Hien, Khuat Thi Thu; Mizutani, Goro; Rutt, Harvey N.
2017-06-01
Asymmetric β-sheet protein structures in spider silk should induce nonlinear optical interaction such as second harmonic generation (SHG) which is experimentally observed for a radial line and dragline spider silk using an imaging femtosecond laser SHG microscope. By comparing different spider silks, we found that the SHG signal correlates with the existence of the protein β-sheets. Measurements of the polarization dependence of SHG from the dragline indicated that the β-sheet has a nonlinear response depending on the direction of the incident electric field. We propose a model of what orientation the β-sheet takes in spider silk.
Nonlinear optical studies of organic monolayers
International Nuclear Information System (INIS)
Shen, Y.R.
1988-02-01
Second-order nonlinear optical effects are forbidden in a medium with inversion symmetry, but are necessarily allowed at a surface where the inversion summary is broken. They are often sufficiently strong so that a submonolayer perturbation of the surface can be readily detected. They can therefore be used as effective tools to study monolayers adsorbed at various interfaces. We discuss here a number of recent experiments in which optical second harmonic generation (SHG) and sum-frequency generation (SFG) are employed to probe and characterize organic monolayers. 15 refs., 5 figs
Optical switching in nonlinear photonic crystals lightly doped with nanostructures
Energy Technology Data Exchange (ETDEWEB)
Singh, Mahi R [Department of Physics and Astronomy, University of Western Ontario, London, ON N6A 3K7 (Canada); Lipson, R H [Department of Chemistry, University of Western Ontario, London, ON N6A 5B7 (Canada)
2008-01-14
A possible switching mechanism has been investigated for nonlinear photonic crystals doped with an ensemble of non-interacting three-level nanoparticles. In this scheme, an intense pump laser field is used to change the refractive index of the nonlinear photonic crystal while a weaker probe field monitors an absorption transition in the nanoparticles. In the absence of the strong laser field the system transmits the probe field when the resonance energy of the nanoparticles lies near the edge of the photonic band gap due to strong coupling between the photonic crystal and the nanoparticles. However, upon application of an intense pump laser field the system becomes absorbing due to a band edge frequency shift that arises due to a nonlinear Kerr effect which changes the refractive index of the crystal. It is anticipated that the optical switching mechanism described in this work can be used to make new types of photonic devices.
Nonlinear optical localization in embedded chalcogenide waveguide arrays
International Nuclear Information System (INIS)
Li, Mingshan; Huang, Sheng; Wang, Qingqing; Chen, Kevin P.; Petek, Hrvoje
2014-01-01
We report the nonlinear optical localization in an embedded waveguide array fabricated in chalcogenide glass. The array, which consists of seven waveguides with circularly symmetric cross sections, is realized by ultrafast laser writing. Light propagation in the chalcogenide waveguide array is studied with near infrared laser pulses centered at 1040 nm. The peak intensity required for nonlinear localization for the 1-cm long waveguide array was 35.1 GW/cm 2 , using 10-nJ pulses with 300-fs pulse width, which is 70 times lower than that reported in fused silica waveguide arrays and with over 7 times shorter interaction distance. Results reported in this paper demonstrated that ultrafast laser writing is a viable tool to produce 3D all-optical switching waveguide circuits in chalcogenide glass
Soil-structure interaction including nonlinear soil
Gicev, Vlado
2008-01-01
There are two types of models of soil-structure system depending upon the rigidity of foundation: models with rigid and models with flexible foundation. Main features of the soil-structure interaction phenomenon: -wave scattering, -radiation damping, -reduction of the system frequencies. In this presentation, the influence of interaction on the development of nonlinear zones in the soil is studied.
Structure/property relationships in non-linear optical materials
Energy Technology Data Exchange (ETDEWEB)
Cole, J M [Institut Max von Laue - Paul Langevin (ILL), 38 - Grenoble (France); [Durham Univ. (United Kingdom); Howard, J A.K. [Durham Univ. (United Kingdom); McIntyre, G J [Institut Max von Laue - Paul Langevin (ILL), 38 - Grenoble (France)
1997-04-01
The application of neutrons to the study of structure/property relationships in organic non-linear optical materials (NLOs) is described. In particular, charge-transfer effects and intermolecular interactions are investigated. Charge-transfer effects are studied by charge-density analysis and an example of one such investigation is given. The study of intermolecular interactions concentrates on the effects of hydrogen-bonding and an example is given of two structurally similar molecules with very disparate NLO properties, as a result of different types of hydrogen-bonding. (author). 3 refs.
Exact solutions for the higher-order nonlinear Schoerdinger equation in nonlinear optical fibres
International Nuclear Information System (INIS)
Liu Chunping
2005-01-01
First, by using the generally projective Riccati equation method, many kinds of exact solutions for the higher-order nonlinear Schoerdinger equation in nonlinear optical fibres are obtained in a unified way. Then, some relations among these solutions are revealed
Nonlinear optical effects in pure and N-doped semiconductors
International Nuclear Information System (INIS)
Donlagic, N.S.
2000-01-01
Over the last decades, the nonlinear optical properties of condensed matter systems have been an attractive and fruitful field of research. While the linear response functions of solids provide information about the elementary excitations of the systems, nonlinear optical experiments give insight into the dynamics of the fundamental many-body processes which are initiated by the external excitations. Stimulated by the experimental results, new theoretical concepts and methods have been developed in order to relate the observed phenomena to the microscopic properties of the investigated materials. The present work deals with the study of the nonlinear dynamics of the optical interband polarization in pure and n-doped semiconductors.In the first part of the thesis, the relaxation behavior of optically excited electron-hole pairs in a one-dimensional semiconductor, which are coupled to longitudinal optical phonons with an initial lattice temperature T>0, is studied with the help of quantum kinetic equations. Apart from Hartree-Fock-like Coulomb contributions, these equations contain additional Coulomb terms, the so-called vertex corrections, by which the influence of the electron-electron interaction on the electron-phonon scattering processes is taken into account. The numerical studies indicate that the vertex corrections are essential for a correct description of the excitonic dynamics.In the second part of the thesis, the attention is shifted to the characteristics of the optical response of a one-dimensional n-doped two-band semiconductor whose conduction band has been linearized with respect to the two Fermi points. Due to the linearization it is possible to calculate the linear and nonlinear response functions of the interacting electron system exactly. These response functions are then used in order to determine the linear absorption spectrum and the time-integrated signal of a degenerated four-wave-mixing experiment. It is shown that the well-known features
Nonlinear optical effects of opening a gap in graphene
Carvalho, David N.; Biancalana, Fabio; Marini, Andrea
2018-05-01
Graphene possesses remarkable electronic, optical, and mechanical properties that have taken the research of two-dimensional relativistic condensed matter systems to prolific levels. However, the understanding of how its nonlinear optical properties are affected by relativisticlike effects has been broadly uncharted. It has been recently shown that highly nontrivial currents can be generated in free-standing samples, notably leading to the generation of even harmonics. Since graphene monolayers are centrosymmetric media, for which such harmonic generation at normal incidence is deemed inaccessible, this light-driven phenomenon is both startling and promising. More realistically, graphene samples are often deposited on a dielectric substrate, leading to additional intricate interactions. Here, we present a treatment to study this instance by gapping the spectrum and we show this leads to the appearance of a Berry phase in the carrier dynamics. We analyze the role of such a phase in the generated nonlinear current and conclude that it suppresses odd-harmonic generation. The pump energy can be tuned to the energy gap to yield interference among odd harmonics mediated by interband transitions, allowing even harmonics to be generated. Our results and general methodology pave the way for understanding the role of gap opening in the nonlinear optics of two-dimensional lattices.
Tunable Resonators for Nonlinear Modal Interactions
Ramini, Abdallah
2016-10-04
Understanding the various mechanisms of nonlinear mode coupling in micro and nano resonators has become an imminent necessity for their successful implementation in practical applications. However, consistent, repeatable, and flexible experimental procedures to produce nonlinear mode coupling are lacking, and hence research into well-controlled experimental conditions is crucial. Here, we demonstrate well-controlled and repeatable experiments to study nonlinear mode coupling among micro and nano beam resonators. Such experimental approach can be applied to other micro and nano structures to help study their nonlinear interactions and exploit them for higher sensitive and less noisy responses. Using electrothermal tuning and electrostatic excitation, we demonstrate three different kinds of nonlinear interactions among the first and third bending modes of vibrations of slightly curved beams (arches): two-one internal resonance, three-one internal resonance, and mode veering (near crossing). The experimental procedure is repeatable, highly flexible, do not require special or precise fabrication, and is conducted in air and at room temperature. This approach can be applied to other micro and nano structures, which come naturally curved due to fabrication imperfections, such as CNTs, and hence lays the foundation to deeply investigate the nonlinear mode coupling in these structures in a consistent way.
Tunable Resonators for Nonlinear Modal Interactions
Ramini, Abdallah; Hajjaj, Amal Z.; Younis, Mohammad I.
2016-01-01
Understanding the various mechanisms of nonlinear mode coupling in micro and nano resonators has become an imminent necessity for their successful implementation in practical applications. However, consistent, repeatable, and flexible experimental procedures to produce nonlinear mode coupling are lacking, and hence research into well-controlled experimental conditions is crucial. Here, we demonstrate well-controlled and repeatable experiments to study nonlinear mode coupling among micro and nano beam resonators. Such experimental approach can be applied to other micro and nano structures to help study their nonlinear interactions and exploit them for higher sensitive and less noisy responses. Using electrothermal tuning and electrostatic excitation, we demonstrate three different kinds of nonlinear interactions among the first and third bending modes of vibrations of slightly curved beams (arches): two-one internal resonance, three-one internal resonance, and mode veering (near crossing). The experimental procedure is repeatable, highly flexible, do not require special or precise fabrication, and is conducted in air and at room temperature. This approach can be applied to other micro and nano structures, which come naturally curved due to fabrication imperfections, such as CNTs, and hence lays the foundation to deeply investigate the nonlinear mode coupling in these structures in a consistent way.
The Quest for the Ultimate Nonlinear Optical Material
Dagenais, M.
1990-10-01
The following sections are included: * Introduction * From Infancy to the Real World * Highly Efficient Nonlinear Optical Materials for Switching and Processing * The Era of Pragmatism * Conclusion * References
Optical Nonlinearities and Ultrafast Carrier Dynamics in Semiconductor Quantum Dots
Energy Technology Data Exchange (ETDEWEB)
Klimov, V.; McBranch, D.; Schwarz, C.
1998-08-10
Low-dimensional semiconductors have attracted great interest due to the potential for tailoring their linear and nonlinear optical properties over a wide-range. Semiconductor nanocrystals (NC's) represent a class of quasi-zero-dimensional objects or quantum dots. Due to quantum cordhement and a large surface-to-volume ratio, the linear and nonlinear optical properties, and the carrier dynamics in NC's are significantly different horn those in bulk materials. napping at surface states can lead to a fast depopulation of quantized states, accompanied by charge separation and generation of local fields which significantly modifies the nonlinear optical response in NC's. 3D carrier confinement also has a drastic effect on the energy relaxation dynamics. In strongly confined NC's, the energy-level spacing can greatly exceed typical phonon energies. This has been expected to significantly inhibit phonon-related mechanisms for energy losses, an effect referred to as a phonon bottleneck. It has been suggested recently that the phonon bottleneck in 3D-confined systems can be removed due to enhanced role of Auger-type interactions. In this paper we report femtosecond (fs) studies of ultrafast optical nonlinearities, and energy relaxation and trap ping dynamics in three types of quantum-dot systems: semiconductor NC/glass composites made by high temperature precipitation, ion-implanted NC's, and colloidal NC'S. Comparison of ultrafast data for different samples allows us to separate effects being intrinsic to quantum dots from those related to lattice imperfections and interface properties.
Nonlinear theory of electroelastic and magnetoelastic interactions
Dorfmann, Luis
2014-01-01
This book provides a unified theory of nonlinear electro-magnetomechanical interactions of soft materials capable of large elastic deformations. The authors include an overview of the basic principles of the classical theory of electromagnetism from the fundamental notions of point charges and magnetic dipoles through to distributions of charge and current in a non-deformable continuum, time-dependent electromagnetic fields and Maxwell’s equations. They summarize the basic ingredients of continuum mechanics that are required to account for the deformability of material and present nonlinear constitutive frameworks for electroelastic and magnetoelastic interactions in a highly deformable material. The equations contained in the book are used to formulate and solve a variety of representative boundary-value problems for both nonlinear electroelasticity and magnetoelasticity.
Linear and nonlinear optical properties of borate crystals as ...
Indian Academy of Sciences (India)
Unknown
crystal series, with an accuracy acceptable for materials development/design, and answer the questions often ... Optical property; nonlinear optical crystals; first principles calculation. 1. ..... system, and is not in concept suitable to excitation pro-.
Non-linear optical imaging – Introduction and pharmaceutical applications
Fussell, A.L.; Isomaki, Antti; Strachan, Clare J.
2013-01-01
Nonlinear optical imaging is an emerging technology with much potential in pharmaceutical analysis. The technique encompasses a range of optical phenomena, including coherent anti-Stokes Raman scattering (CARS), second harmonic generation (SHG), and twophoton excited fluorescence (TPEF). The
Optical polarization based logic functions (XOR or XNOR) with nonlinear Gallium nitride nanoslab.
Bovino, F A; Larciprete, M C; Giardina, M; Belardini, A; Centini, M; Sibilia, C; Bertolotti, M; Passaseo, A; Tasco, V
2009-10-26
We present a scheme of XOR/XNOR logic gate, based on non phase-matched noncollinear second harmonic generation from a medium of suitable crystalline symmetry, Gallium nitride. The polarization of the noncollinear generated beam is a function of the polarization of both pump beams, thus we experimentally investigated all possible polarization combinations, evidencing that only some of them are allowed and that the nonlinear interaction of optical signals behaves as a polarization based XOR. The experimental results show the peculiarity of the nonlinear optical response associated with noncollinear excitation, and are explained using the expression for the effective second order optical nonlinearity in noncollinear scheme.
Nonlinear dynamics of interacting populations
Bazykin, Alexander D
1998-01-01
This book contains a systematic study of ecological communities of two or three interacting populations. Starting from the Lotka-Volterra system, various regulating factors are considered, such as rates of birth and death, predation and competition. The different factors can have a stabilizing or a destabilizing effect on the community, and their interplay leads to increasingly complicated behavior. Studying and understanding this path to greater dynamical complexity of ecological systems constitutes the backbone of this book. On the mathematical side, the tool of choice is the qualitative the
Directory of Open Access Journals (Sweden)
C. Torres-Torres
2012-01-01
Full Text Available We report the transmittance modulation of optical signals in a nanocomposite integrated by two different silver doped zinc oxide thin solid films. An ultrasonic spray pyrolysis approach was employed for the preparation of the samples. Measurements of the third-order nonlinear optical response at a nonresonant 532 nm wavelength of excitation were performed using a vectorial two-wave mixing. It seems that the separated contribution of the optical nonlinearity associated with each film noticeable differs in the resulting nonlinear effects with respect to the additive response exhibited by the bilayer system. An enhancement of the optical Kerr nonlinearity is predicted for prime number arrays of the studied nanoclusters in a two-wave interaction. We consider that the nanostructured morphology of the thin solid films originates a strong modification of the third-order optical phenomena exhibited by multilayer films based on zinc oxide.
Nonlinear interactions of counter-travelling waves
International Nuclear Information System (INIS)
Matsuuchi, Kazuo
1980-01-01
Nonlinear interactions between two waves travelling in opposite directions are investigated. When a nonlinear Klein-Gordon equation is adopted as a model equation, it is shown that such a wave system is governed by a simple set of equations for their complex amplitudes. Steady progressive waves governed by this set are investigated for various cases classified according to the signs of the coefficients. It is then found that one wave travelling in one direction appears from a certain point and the other travelling in the opposite direction has a constant amplitude from that point. This phenomenon may be regarded as a sort of reflection in spite of no rigid boundary. (author)
A Photonic Basis for Deriving Nonlinear Optical Response
Andrews, David L.; Bradshaw, David S.
2009-01-01
Nonlinear optics is generally first presented as an extension of conventional optics. Typically the subject is introduced with reference to a classical oscillatory electric polarization, accommodating correction terms that become significant at high intensities. The material parameters that quantify the extent of the nonlinear response are cast as…
Evaluation of polymer based third order nonlinear integrated optics devices
Driessen, A.; Hoekstra, Hugo; Blom, F.C.; Horst, F.; Horst, F.; Krijnen, Gijsbertus J.M.; van Schoot, J.B.P.; van Schoot, J.B.P.; Lambeck, Paul; Popma, T.J.A.; Diemeer, Mart
Nonlinear polymers are promising materials for high speed active integrated optics devices. In this paper we evaluate the perspectives polymer based nonlinear optical devices can offer. Special attention is directed to the materials aspects. In our experimental work we applied mainly Akzo Nobel DANS
Nonlinear super-resolution nano-optics and applications
Wei, Jingsong
2015-01-01
This book covers many advances in the subjects of nano-optics and nano photonics. The author describes the principle and technical schematics of common methods for breaking through the optical diffraction limit and focuses on realizing optical super-resolution with nonlinear effects of thin film materials. The applications of nonlinear optical super-resolution effects in nano-data storage, nanolithography, and nano-imaging are also presented. This book is useful to graduate students majoring in optics and nano science and also serves as a reference book for academic researchers, engineers, technical professionals in the fields of super-resolution optics and laser techniques, nano-optics and nano photonics, nano-data storage, nano imaging, micro/nanofabrication and nanolithography and nonlinear optics.
Non-Linear Dynamics and Fundamental Interactions
Khanna, Faqir
2006-01-01
The book is directed to researchers and graduate students pursuing an advanced degree. It provides details of techniques directed towards solving problems in non-linear dynamics and chos that are, in general, not amenable to a perturbative treatment. The consideration of fundamental interactions is a prime example where non-perturbative techniques are needed. Extension of these techniques to finite temperature problems is considered. At present these ideas are primarily used in a perturbative context. However, non-perturbative techniques have been considered in some specific cases. Experts in the field on non-linear dynamics and chaos and fundamental interactions elaborate the techniques and provide a critical look at the present status and explore future directions that may be fruitful. The text of the main talks will be very useful to young graduate students who are starting their studies in these areas.
Non-linear soil-structure interaction
International Nuclear Information System (INIS)
Wolf, J.P.
1984-01-01
The basic equation of motion to analyse the interaction of a non-linear structure and an irregular soil with the linear unbounded soil is formulated in the time domain. The contribution of the unbounded soil involves convolution integrals of the dynamic-stiffness coefficients in the time domain and the corresponding motions. As another possibility, a flexibility formulation fot the contribution of the unbounded soil using the dynamic-flexibility coefficients in the time domain, together with the direct-stiffness method for the structure and the irregular soil can be applied. As an example of a non-linear soil-structure-interaction analysis, the partial uplift of the basemat of a structure is examined. (Author) [pt
PREFACE: Ultrafast and nonlinear optics in carbon nanomaterials
Kono, Junichiro
2013-02-01
Carbon-based nanomaterials—single-wall carbon nanotubes (SWCNTs) and graphene, in particular—have emerged in the last decade as novel low-dimensional systems with extraordinary properties. Because they are direct-bandgap systems, SWCNTs are one of the leading candidates to unify electronic and optical functions in nanoscale circuitry; their diameter-dependent bandgaps can be utilized for multi-wavelength devices. Graphene's ultrahigh carrier mobilities are promising for high-frequency electronic devices, while, at the same time, it is predicted to have ideal properties for terahertz generation and detection due to its unique zero-gap, zero-mass band structure. There have been a large number of basic optical studies on these materials, but most of them were performed in the weak-excitation, quasi-equilibrium regime. In order to probe and assess their performance characteristics as optoelectronic materials under device-operating conditions, it is crucial to strongly drive them and examine their optical properties in highly non-equilibrium situations and with ultrashot time resolution. In this section, the reader will find the latest results in this rapidly growing field of research. We have assembled contributions from some of the leading experts in ultrafast and nonlinear optical spectroscopy of carbon-based nanomaterials. Specific topics featured include: thermalization, cooling, and recombination dynamics of photo-generated carriers; stimulated emission, gain, and amplification; ultrafast photoluminescence; coherent phonon dynamics; exciton-phonon and exciton-plasmon interactions; exciton-exciton annihilation and Auger processes; spontaneous and stimulated emission of terahertz radiation; four-wave mixing and harmonic generation; ultrafast photocurrents; the AC Stark and Franz-Keldysh effects; and non-perturbative light-mater coupling. We would like to express our sincere thanks to those who contributed their latest results to this special section, and the
Denz, Cornelia; Simoni, Francesco
2009-03-01
Nonlinearities are becoming more and more important for a variety of applications in nanosciences, bio-medical sciences, information processing and photonics. For applications at the crossings of these fields, especially microscopic and nanoscopic imaging and manipulation, nonlinearities play a key role. They may range from simple nonlinear parameter changes up to applications in manipulating, controlling and structuring material by light, or the manipulation of light by light itself. It is this area between basic nonlinear optics and photonic applications that includes `hot' topics such as ultra-resolution optical microscopy, micro- and nanomanipulation and -structuring, or nanophotonics. This special issue contains contributions in this field, many of them from the International Conference on Nonlinear Microscopy and Optical Control held in conjunction with a network meeting of the ESF COST action MP0604 `Optical Micromanipulation by Nonlinear Nanophotonics', 19-22 February 2008, Münster, Germany. Throughout this special issue, basic investigations of material structuring by nonlinear light--matter interaction, light-induced control of nanoparticles, and novel nonlinear material investigation techniques, are presented, covering the basic field of optical manipulation and control. These papers are followed by impressive developments of optical tweezers. Nowadays, optical phase contrast tweezers, twin and especially multiple beam traps, develop particle control in a new dimension: particles can be arranged, sorted and identified with high throughput. One of the most prominent forthcoming applications of optical tweezers is in the field of microfluidics. The action of light on fluids will open new horizons in microfluidic manipulation and control. The field of optical manipulation and control is a very broad field that has developed in an impressive way, in a short time, in Europe with the installation of the MP0604 network. Top researchers from 19 countries are
Computational studies of third-order nonlinear optical properties of ...
Indian Academy of Sciences (India)
Anuj Kumar
2017-06-20
Jun 20, 2017 ... Department of Physics, Jaypee University of Engineering and Technology, Raghogarh,. Guna 473 226, India. ∗ ... properties and other molecular properties of the organic nonlinear optical crystal 2-aminopyridinium p- toluenesulphonate ... nal processing, optical limiting, optical logic gates, laser radiation ...
Nonlinear Optical Properties of Aluminum Doped Zinc Oxide
Otieno, Calford O.
Nonlinear optical (NLO) materials are crucial to future progress in industrial and technological applications that involve intense light-matter interaction. While ZnO-related materials are known to possess good NLO properties, existing results on ZnO and AZO (Al-doped ZnO) are mostly available at a single wavelength or limited ranges. Therefore, NLO dispersions (wavelength dependences) are not entirely studied, especially at longer wavelengths far below the bandgap. It is important to explore wavelength dependences since doping can induce a drastic change in the NLO responses at varied spectral ranges via doping-induced subgap-state contributions. We present results of our studies on nonlinear harmonic generation from our samples, which include 1) second harmonic generation and 2) third harmonic generation precisely characterized by Maker fringes as a function of both Al doping and wavelength. We exhaustively discuss the possible cause for the modified optical nonlinearities observed in our AZO thin films and give detailed comparisons of our observations with the previous studies. We also present the results of open- and close-aperture Z-scans to characterize the two-photon absorption coefficient (TPA) and the nonlinear refractive index (NLR), respectively, of the AZO films. There was no clearcut evidence of monotonic dependence of TPA and NLR on doping. This presumably indicates that the overall effect is nontrivial and should be understood in terms of combined effects of bandgap shift and crystallinity upon varying the doping level. Most intriguingly, we found that NLR values from the closed-aperture Z-scan are very large by orders of magnitude when compared with the bulk counterparts. Similar observation was made for TPA values from the open-aperture Z-scan. To countercheck very large NLO absorption, we conducted simple intensity scan by varying the incident photon number on each sample but fixing the beam area to eliminate any possible errors related to optical
Nonlinear optical studies of curcumin metal derivatives with cw laser
Energy Technology Data Exchange (ETDEWEB)
Henari, F. Z., E-mail: fzhenari@rcsi-mub.com; Cassidy, S. [Department of Basic Medical Sciences, Royal College of Surgeons in Ireland, Medical University of Bahrain (Bahrain)
2015-03-30
We report on measurements of the nonlinear refractive index and nonlinear absorption coefficients for curcumin and curcumin metal complexes of boron, copper, and iron at different wavelengths using the Z-scan technique. These materials are found to be novel nonlinear media. It was found that the addition of metals slightly influences its nonlinearity. These materials show a large negative nonlinear refractive index of the order of 10{sup −7} cm{sup 2}/W and negative nonlinear absorption of the order of 10{sup −6} cm/W. The origin of the nonlinearity was investigated by comparison of the formalism that is known as the Gaussian decomposition model with the thermal lens model. The optical limiting behavior based on the nonlinear refractive index was also investigated.
Nonlinear optical studies of curcumin metal derivatives with cw laser
International Nuclear Information System (INIS)
Henari, F. Z.; Cassidy, S.
2015-01-01
We report on measurements of the nonlinear refractive index and nonlinear absorption coefficients for curcumin and curcumin metal complexes of boron, copper, and iron at different wavelengths using the Z-scan technique. These materials are found to be novel nonlinear media. It was found that the addition of metals slightly influences its nonlinearity. These materials show a large negative nonlinear refractive index of the order of 10 −7 cm 2 /W and negative nonlinear absorption of the order of 10 −6 cm/W. The origin of the nonlinearity was investigated by comparison of the formalism that is known as the Gaussian decomposition model with the thermal lens model. The optical limiting behavior based on the nonlinear refractive index was also investigated
Coherent Femtosecond Spectroscopy and Nonlinear Optical Imaging on the Nanoscale
Kravtsov, Vasily
Optical properties of many materials and macroscopic systems are defined by ultrafast dynamics of electronic, vibrational, and spin excitations localized on the nanoscale. Harnessing these excitations for material engineering, optical computing, and control of chemical reactions has been a long-standing goal in science and technology. However, it is challenging due to the lack of spectroscopic techniques that can resolve processes simultaneously on the nanometer spatial and femtosecond temporal scales. This thesis describes the fundamental principles, implementation, and experimental demonstration of a novel type of ultrafast microscopy based on the concept of adiabatic plasmonic nanofocusing. Simultaneous spatio-temporal resolution on a nanometer-femtosecond scale is achieved by using a near-field nonlinear optical response induced by ultrafast surface plasmon polaritons nanofocused on a metal tip. First, we study the surface plasmon response in metallic structures and evaluate its prospects and limitations for ultrafast near-field microscopy. Through plasmon emission-based spectroscopy, we investigate dephasing times and interplay between radiative and non-radiative decay rates of localized plasmons and their modification due to coupling. We identify a new regime of quantum plasmonic coupling, which limits the achievable spatial resolution to several angstroms but at the same time provides a potential channel for generating ultrafast electron currents at optical frequencies. Next, we study propagation of femtosecond wavepackets of surface plasmon polaritons on a metal tip. In time-domain interferometric measurements we detect group delays that correspond to slowing of the plasmon polaritons down to 20% of the speed of light at the tip apex. This provides direct experimental verification of the plasmonic nanofocusing mechanism and suggests enhanced nonlinear optical interactions at the tip apex. We then measure a plasmon-generated third-order nonlinear optical
Topology optimization of nonlinear optical devices
DEFF Research Database (Denmark)
Jensen, Jakob Søndergaard
2011-01-01
This paper considers the design of nonlinear photonic devices. The nonlinearity stems from a nonlinear material model with a permittivity that depends on the local time-averaged intensity of the electric field. A finite element model is developed for time-harmonic wave propagation and an incremen......This paper considers the design of nonlinear photonic devices. The nonlinearity stems from a nonlinear material model with a permittivity that depends on the local time-averaged intensity of the electric field. A finite element model is developed for time-harmonic wave propagation...... limiter. Here, air, a linear and a nonlinear material are distributed so that the wave transmission displays a strong sensitivity to the amplitude of the incoming wave....
Ma, Li-Yuan; Ji, Jia-Liang; Xu, Zong-Wei; Zhu, Zuo-Nong
2018-03-01
We study a nonintegrable discrete nonlinear Schrödinger (dNLS) equation with the term of nonlinear nearest-neighbor interaction occurred in nonlinear optical waveguide arrays. By using discrete Fourier transformation, we obtain numerical approximations of stationary and travelling solitary wave solutions of the nonintegrable dNLS equation. The analysis of stability of stationary solitary waves is performed. It is shown that the nonlinear nearest-neighbor interaction term has great influence on the form of solitary wave. The shape of solitary wave is important in the electric field propagating. If we neglect the nonlinear nearest-neighbor interaction term, much important information in the electric field propagating may be missed. Our numerical simulation also demonstrates the difference of chaos phenomenon between the nonintegrable dNLS equation with nonlinear nearest-neighbor interaction and another nonintegrable dNLS equation without the term. Project supported by the National Natural Science Foundation of China (Grant Nos. 11671255 and 11701510), the Ministry of Economy and Competitiveness of Spain (Grant No. MTM2016-80276-P (AEI/FEDER, EU)), and the China Postdoctoral Science Foundation (Grant No. 2017M621964).
Optoelectronic and nonlinear optical processes in low dimensional ...
Indian Academy of Sciences (India)
Optoelectronic process; nonlinear optical process; semiconductor. Quest for ever faster and intelligent information processing technologies has sparked ..... Schematic energy level diagram for the proposed 4-level model. States other than the.
Squeezing in multi-mode nonlinear optical state truncation
International Nuclear Information System (INIS)
Said, R.S.; Wahiddin, M.R.B.; Umarov, B.A.
2007-01-01
In this Letter, we show that multi-mode qubit states produced via nonlinear optical state truncation driven by classical external pumpings exhibit squeezing condition. We restrict our discussions to the two- and three-mode cases
Field-enhanced nonlinear optical properties of organic nanofibers
DEFF Research Database (Denmark)
Kostiučenko, Oksana; Fiutowski, Jacek; Brewer, Jonathan R.
2014-01-01
Second harmonic generation in nonlinearly optically active organic nanofibers, generated via self-assembled surface growth from nonsymmetrically functionalized para-quarterphenylene (CNHP4) molecules, has been investigated. After the growth on mica templates, nanofibers have been transferred onto...
Nonlinear optical beam manipulation, beam combining, and atmospheric propagation
International Nuclear Information System (INIS)
Fischer, R.A.
1988-01-01
These proceedings collect papers on optics: Topics include: diffraction properties of laser speckle, coherent beam combination by plasma modes, nonlinear responses, deformable mirrors, imaging radiometers, electron beam propagation in inhomogeneous media, and stability of laser beams in a structured environment
Nonlinear interaction model of subsonic jet noise.
Sandham, Neil D; Salgado, Adriana M
2008-08-13
Noise generation in a subsonic round jet is studied by a simplified model, in which nonlinear interactions of spatially evolving instability modes lead to the radiation of sound. The spatial mode evolution is computed using linear parabolized stability equations. Nonlinear interactions are found on a mode-by-mode basis and the sound radiation characteristics are determined by solution of the Lilley-Goldstein equation. Since mode interactions are computed explicitly, it is possible to find their relative importance for sound radiation. The method is applied to a single stream jet for which experimental data are available. The model gives Strouhal numbers of 0.45 for the most amplified waves in the jet and 0.19 for the dominant sound radiation. While in near field axisymmetric and the first azimuthal modes are both important, far-field sound is predominantly axisymmetric. These results are in close correspondence with experiment, suggesting that the simplified model is capturing at least some of the important mechanisms of subsonic jet noise.
The chemistry and physics of nonlinear optical materials
International Nuclear Information System (INIS)
Velsko, S.P.; Eimerl, D.
1989-01-01
Recent efforts to engineer new nonlinear optical materials with specific desired characteristics has engendered a need for a theoretical description of optical properties which is readily accessible to chemists, yet correctly treats the essential physics of dielectric response. This paper describes a simple empirical molecular orbital model which gives useful insights into the relationship between chemical composition, crystalline structure, and optical susceptibilities. The authors compare the probabilities of finding new harmonic generators in various chemical classes. Rigorous bounds on the magnitudes of linear and nonlinear optical coefficients and their anisotropies are also discussed
Ultra-Fast Optical Signal Processing in Nonlinear Silicon Waveguides
DEFF Research Database (Denmark)
Oxenløwe, Leif Katsuo; Galili, Michael; Pu, Minhao
2011-01-01
We describe recent demonstrations of exploiting highly nonlinear silicon nanowires for processing Tbit/s optical data signals. We perform demultiplexing and optical waveform sampling of 1.28 Tbit/s and wavelength conversion of 640 Gbit/s data signals.......We describe recent demonstrations of exploiting highly nonlinear silicon nanowires for processing Tbit/s optical data signals. We perform demultiplexing and optical waveform sampling of 1.28 Tbit/s and wavelength conversion of 640 Gbit/s data signals....
Ripple distribution for nonlinear fiber-optic channels.
Sorokina, Mariia; Sygletos, Stylianos; Turitsyn, Sergei
2017-02-06
We demonstrate data rates above the threshold imposed by nonlinearity on conventional optical signals by applying novel probability distribution, which we call ripple distribution, adapted to the properties of the fiber channel. Our results offer a new direction for signal coding, modulation and practical nonlinear distortions compensation algorithms.
Enhancement of nonlinear optical properties of compounds of silica
Indian Academy of Sciences (India)
The aim of this paper is to introduce a method for enhancing the nonlinear optical properties in silica glass by using metallic nanoparticles. First, the T-matrix method is developed to calculate the effective dielectric constant for the compound of silica glass and metallic nanoparticles, both of which possess nonlinear dielectric ...
Nonlinear Fourier transform for dual-polarization optical communication system
DEFF Research Database (Denmark)
Gaiarin, Simone
communication is considered an emerging paradigm in fiber-optic communications that could potentially overcome these limitations. It relies on a mathematical technique called “inverse scattering transform” or “nonlinear Fourier transform (NFT)” to exploit the “hidden” linearity of the nonlinear Schrödinger...
Shahid, Muhammad; Salim, Muhammad; Khalid, Muhammad; Tahir, Muhammad Nawaz; Khan, Muhammad Usman; Braga, Ataualpa Albert Carmo
2018-06-01
In this study, Sulfadiazine-Ortho-Vanillin Schiff base namely (E)-4-((2-hydroxy-3-methoxybenzylidene)amino)sbnd N-(pyrimidin-2-yl)benzene-sulfonamide (BS) was synthesized. Chemical characterization and computational studies using different techniques like XRD, FT-IR, UV-Vis, NBO, FMO, and MEP have been employed. Density functional theory (DFT) calculations have been performed at M06-2X/6-311 + G(d,p) level of theory to obtain optimized geometry and vibrational wave numbers for (E)-4-((2-hydroxy-3-methoxybenzylidene)amino)sbnd N-(pyrimidin-2-yl)benzene-sulfonamide (BS). The DFT optimized geometry supports the experimental XRD parameters. Frontier molecular orbital (FMO) energies and molecular electrostatic potential (MEP) surfaces have been executed at M06-2X/6-311 + G(d,p) level of theory. NBO analysis has been carried out at M06-2X/6-311 + G(d,p) level which not only discovered the hyper conjugative interactions and stability in title molecule but also reconfirmed the existence of Nsbnd H⋯N hydrogen bonds between the dimer. The findings of small EHOMO-ELUMO gap shows less hardness and larger softness values which suggested the bioactiveness of the title molecule. Finally, the effect of solvent on nonlinear optical (NLO) properties has been executed using M06-2X level of theory and 6-311 + G (d,p) basis set. The solvent polarity enhanced the NLO response from 3.62 × 10-30 esu to 4.66 × 10-30 esu indicating the considerable NLO character hence in general may have potential applications in the development of non-linear optical materials.
Effective-medium theory for nonlinear magneto-optics in magnetic granular alloys: cubic nonlinearity
International Nuclear Information System (INIS)
Granovsky, Alexander B.; Kuzmichov, Michail V.; Clerc, J.-P.; Inoue, Mitsuteru
2003-01-01
We propose a simple effective-medium approach for calculating the effective dielectric function of a magnetic metal-insulator granular alloy in which there is a weakly nonlinear relation between electric displacement D and electric field E for both constituent materials of the form D i =ε i (0) E i +χ i (3) |E i | 2 E i . We assume that linear ε i (0) and cubic nonlinear χ i (3) dielectric functions are diagonal and linear with magnetization non-diagonal components. For such metal-insulator composite magneto-optical effects depend on a light intensity and the effective cubic dielectric function χ eff (3) can be significantly greater (up to 10 3 times) than that for constituent materials. The calculation scheme is based on the Bergman and Stroud-Hui theory of nonlinear optical properties of granular matter. The giant cubic magneto-optical nonlinearity is found for composites with metallic volume fraction close to the percolation threshold and at a resonance of optical conductivity. It is shown that a composite may exhibit nonlinear magneto-optics even when both constituent materials have no cubic magneto-optical nonlinearity
Effective-medium theory for nonlinear magneto-optics in magnetic granular alloys: cubic nonlinearity
Energy Technology Data Exchange (ETDEWEB)
Granovsky, Alexander B. E-mail: granov@magn.ru; Kuzmichov, Michail V.; Clerc, J.-P.; Inoue, Mitsuteru
2003-03-01
We propose a simple effective-medium approach for calculating the effective dielectric function of a magnetic metal-insulator granular alloy in which there is a weakly nonlinear relation between electric displacement D and electric field E for both constituent materials of the form D{sub i}={epsilon}{sub i}{sup (0)}E{sub i} +{chi}{sub i}{sup (3)}|E{sub i}|{sup 2}E{sub i}. We assume that linear {epsilon}{sub i}{sup (0)} and cubic nonlinear {chi}{sub i}{sup (3)} dielectric functions are diagonal and linear with magnetization non-diagonal components. For such metal-insulator composite magneto-optical effects depend on a light intensity and the effective cubic dielectric function {chi}{sub eff}{sup (3)} can be significantly greater (up to 10{sup 3} times) than that for constituent materials. The calculation scheme is based on the Bergman and Stroud-Hui theory of nonlinear optical properties of granular matter. The giant cubic magneto-optical nonlinearity is found for composites with metallic volume fraction close to the percolation threshold and at a resonance of optical conductivity. It is shown that a composite may exhibit nonlinear magneto-optics even when both constituent materials have no cubic magneto-optical nonlinearity.
Nonlinear interactions in magnetised piezoelectric semiconductor plasmas
International Nuclear Information System (INIS)
Sharma, Giriraj; Ghosh, S.
2000-01-01
Based on hydrodynamics model of plasmas an analytical investigation of frequency modulational interaction between copropagating high frequency pump and acoustic mode and consequent amplification (steady-state and transient) of the modulated waves is carried out in a magnetised piezoelectric semiconductor medium. The phenomenon of modulation amplification is treated as four wave interaction process involving cubic nonlinearity of the medium. Gain constants, threshold-pump intensities and optimum-pulse duration for the onset of modulational instabilities are estimated. The analysis has been performed in non-dispersive regime of the acoustic mode, which is one of the preconditions for achieving an appreciable initial steady-state growth of the modulated signal wave. It is found that the transient gain diminishes very rapidly if one chooses the pump pulse duration beyond the maximum gain point. Moreover, the desired value of the gain can be obtained by adjusting intensity and pulse duration of the pump and doping concentration of the medium concerned. (author)
Shocks, singularities and oscillations in nonlinear optics and fluid mechanics
Santo, Daniele; Lannes, David
2017-01-01
The book collects the most relevant results from the INdAM Workshop "Shocks, Singularities and Oscillations in Nonlinear Optics and Fluid Mechanics" held in Rome, September 14-18, 2015. The contributions discuss recent major advances in the study of nonlinear hyperbolic systems, addressing general theoretical issues such as symmetrizability, singularities, low regularity or dispersive perturbations. It also investigates several physical phenomena where such systems are relevant, such as nonlinear optics, shock theory (stability, relaxation) and fluid mechanics (boundary layers, water waves, Euler equations, geophysical flows, etc.). It is a valuable resource for researchers in these fields. .
Renormgroup symmetries in problems of nonlinear geometrical optics
International Nuclear Information System (INIS)
Kovalev, V.F.
1996-01-01
Utilization and further development of the previously announced approach [1,2] enables one to construct renormgroup symmetries for a boundary value problem for the system of equations which describes propagation of a powerful radiation in a nonlinear medium in geometrical optics approximation. With the help of renormgroup symmetries new rigorous and approximate analytical solutions of nonlinear geometrical optics equations are obtained. Explicit analytical expressions are presented that characterize spatial evolution of laser beam which has an arbitrary intensity dependence at the boundary of the nonlinear medium. (author)
Nonlinear atom optics and bright-gap-soliton generation in finite optical lattices
International Nuclear Information System (INIS)
Carusotto, Iacopo; Embriaco, Davide; La Rocca, Giuseppe C.
2002-01-01
We theoretically investigate the transmission dynamics of coherent matter wave pulses across finite optical lattices in both the linear and the nonlinear regimes. The shape and the intensity of the transmitted pulse are found to strongly depend on the parameters of the incident pulse, in particular its velocity and density: a clear physical picture of the main features observed in the numerical simulations is given in terms of the atomic band dispersion in the periodic potential of the optical lattice. Signatures of nonlinear effects due to the atom-atom interaction are discussed in detail, such as atom-optical limiting and atom-optical bistability. For positive scattering lengths, matter waves propagating close to the top of the valence band are shown to be subject to modulational instability. A scheme for the experimental generation of narrow bright gap solitons from a wide Bose-Einstein condensate is proposed: the modulational instability is seeded starting from the strongly modulated density profile of a standing matter wave and the solitonic nature of the generated pulses is checked from their shape and their collisional properties
Achieving nonlinear optical modulation via four-wave mixing in a four-level atomic system
Li, Hai-Chao; Ge, Guo-Qin; Zubairy, M. Suhail
2018-05-01
We propose an accessible scheme for implementing tunable nonlinear optical amplification and attenuation via a synergetic mechanism of four-wave mixing (FWM) and optical interference in a four-level ladder-type atomic system. By constructing a cyclic atom-field interaction, we show that two reverse FWM processes can coexist via optical transitions in different branches. In the suitable input-field conditions, strong interference effects between the input fields and the generated FWM fields can be induced and result in large amplification and deep attenuation of the output fields. Moreover, such an optical modulation from enhancement to suppression can be controlled by tuning the relative phase. The quantum system can be served as a switchable optical modulator with potential applications in quantum nonlinear optics.
Nonlinear optics response of semiconductor quantum wells under high magnetic fields
International Nuclear Information System (INIS)
Chemla, D.S.
1993-07-01
Recent investigations on the nonlinear optical response of semiconductor quantum wells in a strong perpendicular magnetic field, H, are reviewed. After some introductory material the evolution of the linear optical properties of GaAs QW's as a function of H is discussed; an examination is made of how the magneto-excitons (MX) extrapolate continuously between quasi-2D QW excitons (X) when H = 0, and pairs of Landau levels (LL) when H → ∞. Next, femtosecond time resolved investigations of their nonlinear optical response are presented; the evolution of MX-MX interactions with increasing H is stressed. Finally, how, as the dimensionality is reduced by application of H, the number of scattering channels is limited and relaxation of electron-hole pairs is affected. How nonlinear optical spectroscopy can be exploited to access the relaxation of angular momentum within magneto-excitons is also discussed
Second-order nonlinear optical metamaterials: ABC-type nanolaminates
International Nuclear Information System (INIS)
Alloatti, L.; Kieninger, C.; Lauermann, M.; Köhnle, K.; Froelich, A.; Wegener, M.; Frenzel, T.; Freude, W.; Leuthold, J.; Koos, C.
2015-01-01
We demonstrate a concept for second-order nonlinear metamaterials that can be obtained from non-metallic centrosymmetric constituents with inherently low optical absorption. The concept is based on iterative atomic-layer deposition of three different materials, A = Al 2 O 3 , B = TiO 2 , and C = HfO 2 . The centrosymmetry of the resulting ABC stack is broken since the ABC and the inverted CBA sequences are not equivalent—a necessary condition for non-zero second-order nonlinearity. In our experiments, we find that the bulk second-order nonlinear susceptibility depends on the density of interfaces, leading to a nonlinear susceptibility of 0.26 pm/V at a wavelength of 800 nm. ABC-type nanolaminates can be deposited on virtually any substrate and offer a promising route towards engineering of second-order optical nonlinearities at both infrared and visible wavelengths
Linear and non-linear optics of condensed matter
International Nuclear Information System (INIS)
McLean, T.P.
1977-01-01
Part I - Linear optics: 1. General introduction. 2. Frequency dependence of epsilon(ω, k vector). 3. Wave-vector dependence of epsilon(ω, k vector). 4. Tensor character of epsilon(ω, k vector). Part II - Non-linear optics: 5. Introduction. 6. A classical theory of non-linear response in one dimension. 7. The generalization to three dimensions. 8. General properties of the polarizability tensors. 9. The phase-matching condition. 10. Propagation in a non-linear dielectric. 11. Second harmonic generation. 12. Coupling of three waves. 13. Materials and their non-linearities. 14. Processes involving energy exchange with the medium. 15. Two-photon absorption. 16. Stimulated Raman effect. 17. Electro-optic effects. 18. Limitations of the approach presented here. (author)
Ageing of the nonlinear optical susceptibility in soft matter
International Nuclear Information System (INIS)
Ghofraniha, N; Conti, C; Leonardo, R Di; Ruzicka, B; Ruocco, G
2007-01-01
We investigate the nonlinear optics response of a colloidal dispersion undergoing dynamics slowing down with age, by using Z-scan and dynamic light scattering measurements. We study the high optical nonlinearity of an organic dye (rhodamine B) dispersed in a water-clay (laponite) suspension. We consider different clay concentrations (2.0-2.6 wt%) experiencing dynamics arrest. We find that (i) the concentration dependent exponential growth of both mean relaxation time and nonlinear absorption coefficient can be individually scaled to a master curve and (ii) the scaling times are the same for the two physical quantities. These findings indicate that the optical nonlinear susceptibility exhibits the same ageing universal scaling behaviour, typical of disordered out of equilibrium systems
A variational approach to nonlinear evolution equations in optics
Indian Academy of Sciences (India)
optics. D ANDERSON, M LISAK and A BERNTSON£. Department of Electromagnetics, Chalmers University of Technology, SE-41296 Göteborg, Sweden. £Ericsson Telcom ... Many works in nonlinear optics have made efficient ...... focusing dynamics of a laser beam (or a Bose–Einstein condensate) in a parabolic external.
Nonlinear Optics: Materials, Fundamentals, and Applications. Postdeadline papers
1992-08-01
The Nonlinear Optics: Materials, Fundamentals, and Applications conference was held on 17-21 Aug. 1992. The following topics were addressed: subpicosecond time resolved four-wave mixing spectroscopy in heteroepitaxial ZnSe thin layers; anisotropic two-photon transition in GaAs/AlGaAs multiple quantum well waveguides; two picosecond, narrow-band, tunable, optical parametric systems using BBO and LBO; second generation in an optically active liquid: experimental observation of a fourth-order optical nonlinearity due to molecular chirality; optical image recognition system implemented with a 3-D memory disk; phase-matched second-harmonic generation in waveguides of polymeric Langmuir-Blodgett films; fluence dependent dynamics observed in the resonant third-order optical response of C60 and C70 films; temporal modulation of spatial optical solitons: a variational approach; measurements of light-scattering noise during two-wave mixing in a Kerr medium; excess noise introduced by beam propagation through an atomic vapor; an approach to all-optical switching based on second-order nonlinearities; multilayer, nonlinear ARROW waveguides for surface emitted sum-frequency mixing; energy scaling of SBS phase conjugate mirrors to 4J; vector versus scalar theory for the double phase conjugate mirror; cross-talk and error probability in counter-beam lambda-multiplexed digital holograms; and modal growth of SHG in doped silica thin film waveguides.
Nonlinear fiber-optic strain sensor based on four-wave mixing in microstructured optical fiber
DEFF Research Database (Denmark)
Gu, Bobo; Yuan, Scott Wu; Frosz, Michael H.
2012-01-01
We demonstrate a nonlinear fiber-optic strain sensor, which uses the shifts of four-wave mixing Stokes and anti-Stokes peaks caused by the strain-induced changes in the structure and refractive index of a microstructured optical fiber. The sensor thus uses the inherent nonlinearity of the fiber a...
Nonlinear optical properties of ultrathin metal layers
DEFF Research Database (Denmark)
Lysenko, Oleg
2016-01-01
This thesis presents experimental and theoretical studies of nonlinear propagation of ultrashort long-range surface plasmon polaritons in gold strip waveguides. The strip plasmonic waveguides are fabricated in house, and contain a gold layer, adhesion layers, and silicon dioxide cladding. The opt......This thesis presents experimental and theoretical studies of nonlinear propagation of ultrashort long-range surface plasmon polaritons in gold strip waveguides. The strip plasmonic waveguides are fabricated in house, and contain a gold layer, adhesion layers, and silicon dioxide cladding......-order nonlinear susceptibility of the plasmonic mode in the gold strip waveguides significantly depends on the metal layer thickness and laser pulse duration. This dependence is explained in detail in terms of the free-electron temporal dynamics in gold. The third-order nonlinear susceptibility of the gold layer...
Nonboson treatment of excitonic nonlinearity in optically excited media
International Nuclear Information System (INIS)
Nguyen Ba An.
1990-11-01
The present article shortly reviews some recent results in the study of excitonic nonlinearity in optically excited media using a nonboson treatment for many-exciton systems. After a brief discussion of the exciton nonbosonity the closed commutation relations are given for exciton operators which hold for any exciton density and type. The nonboson treatment is then applied to the problems of intrinsic optical bistability and nonlinear polariton yielding quite interesting and new effects, e.g. new shapes of hysteresis loops of intrinsic optical bistability or anomalies of polariton dispersion. (author). 71 refs, 4 figs
DEFF Research Database (Denmark)
Bache, Morten; Bang, Ole; Zhou, Binbin
2011-01-01
When ultrafast noncritical cascaded second-harmonic generation of energetic femtosecond pulses occur in a bulk lithium niobate crystal optical Cherenkov waves are formed in the near- to mid-IR. Numerical simulations show that the few-cycle solitons radiate Cherenkov (dispersive) waves in the λ = 2...
Hofstadter butterflies in nonlinear Harper lattices, and their optical realizations
International Nuclear Information System (INIS)
Manela, Ofer; Segev, Mordechai; Christodoulides, Demetrios N; Kip, Detlef
2010-01-01
The ubiquitous Hofstadter butterfly describes a variety of systems characterized by incommensurable periodicities, ranging from Bloch electrons in magnetic fields and the quantum Hall effect to cold atoms in optical lattices and more. Here, we introduce nonlinearity into the underlying (Harper) model and study the nonlinear spectra and the corresponding extended eigenmodes of nonlinear quasiperiodic systems. We show that the spectra of the nonlinear eigenmodes form deformed versions of the Hofstadter butterfly and demonstrate that the modes can be classified into two families: nonlinear modes that are a 'continuation' of the linear modes of the system and new nonlinear modes that have no counterparts in the linear spectrum. Finally, we propose an optical realization of the linear and nonlinear Harper models in transversely modulated waveguide arrays, where these Hofstadter butterflies can be observed. This work is relevant to a variety of other branches of physics beyond optics, such as disorder-induced localization in ultracold bosonic gases, localization transition processes in disordered lattices, and more.
Hofstadter butterflies in nonlinear Harper lattices, and their optical realizations
Energy Technology Data Exchange (ETDEWEB)
Manela, Ofer; Segev, Mordechai [Department of Physics and Solid State Institute, Technion, Haifa 32000 (Israel); Christodoulides, Demetrios N [College of Optics/CREOL, University of Central Florida, FL 32816-2700 (United States); Kip, Detlef, E-mail: msegev@tx.technion.ac.i [Department of Electrical Engineering, Helmut Schmidt University, 22043 Hamburg (Germany)
2010-05-15
The ubiquitous Hofstadter butterfly describes a variety of systems characterized by incommensurable periodicities, ranging from Bloch electrons in magnetic fields and the quantum Hall effect to cold atoms in optical lattices and more. Here, we introduce nonlinearity into the underlying (Harper) model and study the nonlinear spectra and the corresponding extended eigenmodes of nonlinear quasiperiodic systems. We show that the spectra of the nonlinear eigenmodes form deformed versions of the Hofstadter butterfly and demonstrate that the modes can be classified into two families: nonlinear modes that are a 'continuation' of the linear modes of the system and new nonlinear modes that have no counterparts in the linear spectrum. Finally, we propose an optical realization of the linear and nonlinear Harper models in transversely modulated waveguide arrays, where these Hofstadter butterflies can be observed. This work is relevant to a variety of other branches of physics beyond optics, such as disorder-induced localization in ultracold bosonic gases, localization transition processes in disordered lattices, and more.
Shen, Yujia; Wen, Zichao; Yan, Zhenya; Hang, Chao
2018-04-01
We study the three-wave interaction that couples an electromagnetic pump wave to two frequency down-converted daughter waves in a quadratic optical crystal and P T -symmetric potentials. P T symmetric potentials are shown to modulate stably nonlinear modes in two kinds of three-wave interaction models. The first one is a spatially extended three-wave interaction system with odd gain-and-loss distribution in the channel. Modulated by the P T -symmetric single-well or multi-well Scarf-II potentials, the system is numerically shown to possess stable soliton solutions. Via adiabatical change of system parameters, numerical simulations for the excitation and evolution of nonlinear modes are also performed. The second one is a combination of P T -symmetric models which are coupled via three-wave interactions. Families of nonlinear modes are found with some particular choices of parameters. Stable and unstable nonlinear modes are shown in distinct families by means of numerical simulations. These results will be useful to further investigate nonlinear modes in three-wave interaction models.
Kohlgraf-Owens, Dana C; Kik, Pieter G
2009-08-17
The linear and nonlinear optical properties of a composite containing interacting spherical silver nanoparticles embedded in a dielectric host are studied as a function of interparticle separation using three dimensional frequency domain simulations. It is shown that for a fixed amount of metal, the effective third-order nonlinear susceptibility of the composite chi((3))(omega) can be significantly enhanced with respect to the linear optical properties, due to a combination of resonant surface plasmon excitation and local field redistribution. It is shown that this geometry-dependent susceptibility enhancement can lead to an improved figure of merit for nonlinear absorption. Enhancement factors for the nonlinear susceptibility of the composite are calculated, and the complex nature of the enhancement factors is discussed.
A nonlinear plasmonic waveguide based all-optical bidirectional switching
Bana, Xiaoqiang; Pang, Xingxing; Li, Xiaohui; Hu, Bin; Guo, Yixuan; Zheng, Hairong
2018-01-01
In this paper, an all-optical switching with a nanometer coupled ring resonator is demonstrated based on the nonlinear material. By adjusting the light intensity, we implement the resonance wavelength from 880 nm to 940 nm in the nonlinear material structure monocyclic. In the bidirectional switch structure, the center wavelength (i.e. 880 nm) is fixed. By changing the light intensity from I = 0 to I = 53 . 1 MW /cm2, the function of optical switching can be obtained. The results demonstrate that both the single-ring cavity and the T-shaped double-ring structure can realize the optical switching effect. This work takes advantage of the simple structure. The single-ring cavity plasmonic switches have many advantages, such as nanoscale size, low pumping light intensity, ultrafast response time (femtosecond level), etc. It is expected that the proposed all-optical integrated devices can be potentially applied in optical communication, signal processing, and signal sensing, etc.
Nonlinear optical studies of single gold nanoparticles
Dijk, Meindert Alexander van
2007-01-01
Gold nanoparticles are spherical clusters of gold atoms, with diameters typically between 1 and 100 nanometers. The applications of these particles are rather diverse, from optical labels for biological experiments to data carrier for optical data storage. The goal of my project was to develop new
Label-free and selective nonlinear fiber-optical biosensing
DEFF Research Database (Denmark)
Ott, Johan Raunkjær; Heuck, Mikkel; Agger, Christian
2008-01-01
We demonstrate that the inherent nonlinearity of a microstructured optical fiber (MOF) may be used to achieve label-free selective biosensing, thereby eliminating the need for post-processing of the fiber. This first nonlinear biosensor utilizes a change in the modulational instability (MI) gain...... for optimizing the sensitivity. The nonlinear sensor shows a sensitivity of around 10.4nm/nm, defined as the shift in resonance wavelength per nm biolayer, which is a factor of 7.5 higher than the hitherto only demonstrated label-free MOF biosensor....
Hu, Ming-Lie; Wang, Ching-Yue; Song, You-Jian; Li, Yan-Feng; Chai, Lu; Serebryannikov, Evgenii; Zheltikov, Aleksei
2006-02-06
We demonstrate an experimental technique that allows a mapping of vectorial nonlinear-optical processes in multimode photonic-crystal fibers (PCFs). Spatial and polarization modes of PCFs are selectively excited in this technique by varying the tilt angle of the input beam and rotating the polarization of the input field. Intensity spectra of the PCF output plotted as a function of the input field power and polarization then yield mode-resolved maps of nonlinear-optical interactions in multimode PCFs, facilitating the analysis and control of nonlinear-optical transformations of ultrashort laser pulses in such fibers.
Picosecond optical nonlinearities in symmetrical and unsymmetrical ...
Indian Academy of Sciences (India)
It is evident that the saturable absorption (SA) behaviour changed to reverse sat- urable absorption (RSA) and the nonlinear coefficients were obtained using the equation α = α0I/[1 + (I/Is)]. The open-aperture scans were fitted by solving the propagation equation for homogeneous medium dI/dz = {−α0I/[1+(I/Is)]}−βI2.
Optical computation based on nonlinear total reflectional optical ...
Indian Academy of Sciences (India)
Optical computing; beam splitter; optical switch; polarized beams. ... main research direction called quantum information and quantum computation is .... above has several advantages: Firstly, it is easy to be integrated with appropriate.
Transverse effects in nonlinear optics: Toward the photon superfluid
McCormick, Colin Fraser
Nonlinear optics displays a wealth of transverse effects. These effects are particularly rich in the presence of an optical cavity. Many considerations suggest that in a Kerr nonlinear cavity a new state of light known as a "photon superfluid" can form, with strong analogies to atomic superfluids. The conditions for the formation of the photon superfluid include requirements on the cavity, input light fields and the nonlinear medium as well as various timescales. The most favorable candidate nonlinear medium for observing the photon super-fluid is an atomic vapor. With a strong and fast Kerr effect, atomic vapors also have the advantage of a Kerr coefficient that is tunable in both magnitude and sign. A series of z-scan experiments in far-detuned atomic rubidium vapor is reported, measuring the Kerr coefficient and determining its functional dependence on detuning to be that of a Doppler-broadened two-level model with adiabatic following of the electric field by the atom pseudomoment. Saturation effects are found to be important. Z-scan measurements for detunings within the Doppler profile are shown to agree well with numerical simulations based on the Doppler-broadened model. Agreement between absorptive and refractive non-linear coefficients is evidence of the Kramers-Kronig relations at work, even in this nonlinear system. The formation of the photon superfluid is discussed and the calculation of a new process, nearly collinear four-wave mixing, is presented. This process is essentially an inverse beam filamentation that is likely to be the underlying physical mechanism for transverse cooling and condensation of photons in a nonlinear optical cavity. Nearly collinear four-wave mixing may also be related to phenomena in general nonlinear physics, including modulation instability and Fermi-Pasta-Ulam recurrence.
Wu, Xingzhi; Xiao, Jinchong; Sun, Ru; Jia, Jidong; Yang, Junyi; Ao, Guanghong; Shi, Guang; Wang, Yuxiao; Zhang, Xueru; Song, Yinglin
2018-06-01
Spindle-type molecules containing twisted acenes (PyBTA-1 &PyBTA-2) are designed, synthesized characterized. Picosecond Z-scan experiments under 532 nm show reverse saturable absorption and negative nonlinear refraction, indicating large third-order optical nonlinearity in PyBTA-1. The mechanism of the optical nonlinearity is investigated and the results show that the nonlinear absorption and refraction in PyBTA-1 originates from a charge transfer (CT) state. Furthermore, relatively long lifetime and absorptive cross section of the CT state are measured. Based on the excited state absorption in PyBTA-1, strong optical limiting with ∼0.3 J/cm2 thresholds are obtained when excited by picoseconds and nanoseconds pulses. The findings on nonlinear optics suggest PyBTA-1 a promising material of all optical modulation and laser protection, which enrich the potential applications of these spindle-type molecules. Comparing to the previously reported spindle-type molecules with analogous structures, the introduction of ICT in PyBTA-1 &PyBTA-2 dramatically decreases the two-photon absorption while enhances the nonlinear refraction. The results could be used to selectively tailor the optical nonlinearity in such kind of compounds.
Nonlinear Fourier transform for dual-polarization optical communication system
Gaiarin, Simone
2018-01-01
New services and applications are causing an exponential increase in the internet traffic. In a few years, the current fiber-optic communication system infrastructure will not be able to meet this demand because fiber nonlinearity dramatically limits the information transmission rate. Eigenvalue communication is considered an emerging paradigm in fiber-optic communications that could potentially overcome these limitations. It relies on a mathematical technique called “inverse scattering trans...
Theory of plasmonic effects in nonlinear optics: the case of graphene
Rostami, Habib; Katsnelson, Mikhail I.; Polini, Marco; Mikhail I. Katsnelson Collaboration; Habib Rostami; Marco Polini Collaboration
The nonlinear optical properties of two-dimensional electronic systems are beginning to attract considerable interest both in the theoretical and experimental sectors. Recent experiments on the nonlinear optical properties of graphene reveal considerably strong third harmonic generation and four-wave mixing of this single-atomic-layer electronic system. We develop a large-N theory of electron-electron interaction corrections to multi-legged Feynman diagrams describing second- and third-order nonlinear response functions. Our theory is completely general and is useful to understand all second- and third-order nonlinear effects, including harmonic generation, wave mixing, and photon drag. We apply our theoretical framework to the case of graphene, by carrying out microscopic calculations of the second- and third-order nonlinear response functions of an interacting two-dimensional gas of massless Dirac fermions. We compare our results with recent measurements, where all-optical launching of graphene plasmons has been achieved. This work was supported by Fondazione Istituto Italiano di Tecnologia, the European Union's Horizon 2020 research and innovation programme under Grant agreement No. 696656 GrapheneCore, and the ERC Advanced Grant 338957 FEMTO/NANO (M.I.K.).
Optical Beams in Nonlocal Nonlinear Media
DEFF Research Database (Denmark)
Królikowski, W.; Bang, Ole; Wyller, J.
2003-01-01
We discuss propagation of optical beams in nonlocal Kerr-like media with the nonlocality of general form. We study the effect of nonlocality on modulational instability of the plane wave fronts, collapse of finite beams and formation of spatial solitons....
Nonlinear optical studies in semiconductor-doped glasses under ...
Indian Academy of Sciences (India)
Abstract. Nonlinear optical studies in semiconductor-doped glasses (SDGs) are per- formed under femtosecond laser pulse excitation. Z-scan experiments with 800 nm wave- length pulses are used to excite SDG samples in the resonance and non-resonance regimes. Schott colour glass filter OG 515 shows stronger ...
Nonlinear Optics Approaches Towards Subdiffraction Resolution in CARS Imaging
Boller, Klaus J.; Beeker, W.P.; Cleff, C.; Kruse, K.; Lee, Christopher James; Gross, P.; Offerhaus, Herman L.; Fallnich, Carsten; Herek, Jennifer Lynn; Fornasiero, E.F.; Rizzoli, S.O.
2014-01-01
In theoretical investigations, we review several nonlinear optical approaches towards subdiffraction-limited resolution in label-free imaging via coherent anti-Stokes Raman scattering (CARS). Using a density matrix model and numerical integration, we investigate various level schemes and
Enhancement of nonlinear optical properties of compounds of silica ...
Indian Academy of Sciences (India)
Enhancement of nonlinear optical properties of compounds of silica glass and metallic nanoparticle. A GHARAATI1,∗ and A KAMALDAR1,2. 1Department of Physics, Payame Noor University, P.O. Box 19395-3697, Tehran, Iran. 2Department of Education 1, Shiraz, Iran. ∗. Corresponding author. E-mail: agharaati@pnu.ac.
Printed organic smart devices characterized by nonlinear optical
DEFF Research Database (Denmark)
Pastorelli, Francesco; Accanto, Nicolo; Jørgensen, Mikkel
2017-01-01
In this study, we demonstrate that nonlinear optical microscopy is a promising technique to characterize organic printed electronics. Using ultrashort laser pulses we stimulate two-photon absorption in a roll coated polymer semiconductor and map the resulting two-photon induced photoluminescence...
Optical activity via Kerr nonlinearity in a spinning chiral medium
Energy Technology Data Exchange (ETDEWEB)
Khan, Anwar Ali, E-mail: anwarali@uom.edu.pk [Department of Physics, University of Malakand at Chakdara Dir(L) (Pakistan); Bacha, Bakht Amin, E-mail: aminoptics@gmail.com [Department of Physics, University of Malakand at Chakdara Dir(L) (Pakistan); Khan, Rahmat Ali, E-mail: rahmat_alipk@yahoo.com [Department of Mathematics, University of Malakand (Pakistan)
2016-11-11
Optical activity is investigated in a chiral medium by employing the four level cascade atomic model, in which the optical responses of the atomic medium are studied with Kerr nonlinearity. Light entering into a chiral medium splits into circular birefringent beams. The angle of divergence between the circular birefringent beams and the polarization states of the two light beams is manipulated with Kerr nonlinearity. In the stationary chiral medium the angle of divergence between the circular birefringent beams is calculated to be 1.3 radian. Furthermore, circular birefringence is optically controlled in a spinning chiral medium, where the maximum rotary photon drag angle for left (right) circularly polarized beam is ±1.1 (±1.5) microradian. The change in the angle of divergence between circular birefringent beams by rotary photon drag is calculated to be 0.4 microradian. The numerical results may help to understand image designing, image coding, discovery of photonic crystals and optical sensing technology. - Highlights: • Coherent control of a circular birefringence in a chiral medium is studied. • Angle of divergence between birefringent beams is modified with Kerr nonlinearity. • Rotary photon drag is controlled for birefringent beams and enhanced with Kerr nonlinearity in a spinning medium. • Rotation of the angle of divergence is observed with mechanical rotation of the medium about an axis and modified with Kerr effect. • A change in the angle of divergence is calculated by about a microradian with rotary photon drag.
Extra phase noise from thermal fluctuations in nonlinear optical crystals
DEFF Research Database (Denmark)
César, J. E. S.; Coelho, A.S.; Cassemiro, K.N.
2009-01-01
We show theoretically and experimentally that scattered light by thermal phonons inside a second-order nonlinear crystal is the source of additional phase noise observed in optical parametric oscillators. This additional phase noise reduces the quantum correlations and has hitherto hindered the d...
Generalized dispersive wave emission in nonlinear fiber optics.
Webb, K E; Xu, Y Q; Erkintalo, M; Murdoch, S G
2013-01-15
We show that the emission of dispersive waves in nonlinear fiber optics is not limited to soliton-like pulses propagating in the anomalous dispersion regime. We demonstrate, both numerically and experimentally, that pulses propagating in the normal dispersion regime can excite resonant dispersive radiation across the zero-dispersion wavelength into the anomalous regime.
Lossy effects in a nonlinear nematic optical fiber
Rodríguez, R. F.; Reyes, J. A.
2001-09-01
We use the multiple scales method to derive a generalized nonlinear Schrödinger equation that takes into account the dissipative effects in the reorientation of a nematic confined in a cylindrical waveguide. This equation has soliton-like solutions and predicts a decrease in the penetration length of the optical solitons for each propagating mode with respect to the dissipationless case.
Linear and nonlinear optical spectroscopy: Spectral, temporal and spatial resolution
DEFF Research Database (Denmark)
Hvam, Jørn Marcher
1997-01-01
Selected linear and nonlinear optical spectroscopies are being described with special emphasis on the possibility of obtaining simultaneous spectral, temporal and spatial resolution. The potential of various experimental techniques is being demonstrated by specific examples mostly taken from inve...... investigations of the electronic, and opto-electronic, properties of semiconductor nanostructures....
Applied nonlinear optics in the journal 'Quantum Electronics'
International Nuclear Information System (INIS)
Grechin, Sergei G; Dmitriev, Valentin G; Chirkin, Anatolii S
2011-01-01
A brief historical review of the experimental and theoretical works on nonlinear optical frequency conversion (generation of harmonics, up- and down-conversion, parametric oscillation), which have been published in the journal 'Quantum Electronics' for the last 40 years, is presented.
Instrumentation for Linear and Nonlinear Optical Device Characterization
2018-01-31
distribution is Unlimited 13. SUPPLEMENTARY NOTES 14. ABSTRACT The Pl has acquired six pieces of equipment to extend capabilities for linear and nonlinear...optical spectral analysis • Frequency comb generation in mid-infrared Accomplishments Six major pieces of equipment have been ordered and received
Interaction of few-cycle laser pulses in an isotropic nonlinear medium
International Nuclear Information System (INIS)
Oganesyan, D L; Vardanyan, A O
2007-01-01
The interaction of few-cycle laser pulses propagating in an isotropic nonlinear medium is studied theoretically. A system of nonlinear Maxwell's equations is integrated numerically with respect to time by the finite difference method. The interaction of mutually orthogonal linearly polarised 0.81-μm, 10-fs pulses is considered. Both the instant Kerr polarisation response and Raman inertial response of the medium in the nonlinear part of the medium are taken into account. The spectral shift of the probe pulse caused by the cross-action of the reference pulse is studied. The spectra of the interacting pulses are studied for different time delays between them and the shifts of these spectra are obtained as a function of the time delay. (nonlinear optical phenomena)
Tangled nonlinear driven chain reactions of all optical singularities
Vasil'ev, V. I.; Soskin, M. S.
2012-03-01
Dynamics of polarization optical singularities chain reactions in generic elliptically polarized speckle fields created in photorefractive crystal LiNbO3 was investigated in details Induced speckle field develops in the tens of minutes scale due to photorefractive 'optical damage effect' induced by incident beam of He-Ne laser. It was shown that polarization singularities develop through topological chain reactions of developing speckle fields driven by photorefractive nonlinearities induced by incident laser beam. All optical singularities (C points, optical vortices, optical diabolos,) are defined by instantaneous topological structure of the output wavefront and are tangled by singular optics lows. Therefore, they have develop in tangled way by six topological chain reactions driven by nonlinear processes in used nonlinear medium (photorefractive LiNbO3:Fe in our case): C-points and optical diabolos for right (left) polarized components domains with orthogonally left (right) polarized optical vortices underlying them. All elements of chain reactions consist from loop and chain links when nucleated singularities annihilated directly or with alien singularities in 1:9 ratio. The topological reason of statistics was established by low probability of far enough separation of born singularities pair from existing neighbor singularities during loop trajectories. Topology of developing speckle field was measured and analyzed by dynamic stokes polarimetry with few seconds' resolution. The hierarchy of singularities govern scenario of tangled chain reactions was defined. The useful space-time data about peculiarities of optical damage evolution were obtained from existence and parameters of 'islands of stability' in developing speckle fields.
Progress in linear optics, non-linear optics and surface alignment of liquid crystals
Ong, H. L.; Meyer, R. B.; Hurd, A. J.; Karn, A. J.; Arakelian, S. M.; Shen, Y. R.; Sanda, P. N.; Dove, D. B.; Jansen, S. A.; Hoffmann, R.
We first discuss the progress in linear optics, in particular, the formulation and application of geometrical-optics approximation and its generalization. We then discuss the progress in non-linear optics, in particular, the enhancement of a first-order Freedericksz transition and intrinsic optical bistability in homeotropic and parallel oriented nematic liquid crystal cells. Finally, we discuss the liquid crystal alignment and surface effects on field-induced Freedericksz transition.
Matsuda, Nobuyuki; Kato, Takumi; Harada, Ken-Ichi; Takesue, Hiroki; Kuramochi, Eiichi; Taniyama, Hideaki; Notomi, Masaya
2011-10-10
We demonstrate highly enhanced optical nonlinearity in a coupled-resonator optical waveguide (CROW) in a four-wave mixing experiment. Using a CROW consisting of 200 coupled resonators based on width-modulated photonic crystal nanocavities in a line defect, we obtained an effective nonlinear constant exceeding 10,000 /W/m, thanks to slow light propagation combined with a strong spatial confinement of light achieved by the wavelength-sized cavities.
Interaction-induced effects in the nonlinear coherent response of quantum-well excitons
DEFF Research Database (Denmark)
Wagner, Hans Peter; Schätz, A.; Langbein, Wolfgang Werner
1999-01-01
Interaction-induced processes are studied using the third-order nonlinear polarization created in polarization-dependent four-wave-mixing experiments (FWM) on a ZnSe single quantum well. We discuss their influence by a comparison of the experimental FWM with calculations based on extended optical...
Materials for Nonlinear Optics Chemical Perspectives
1991-01-01
potassium iodide for 15 h at reflux. The benzaldehyde product was then allowed to react with diethyl(4-nitrobenzyl)phosphonate in the presence of ...photocrosslinking of NLO-inactive polyacrylate monomers. Recent advances in optical technology have created great interest in the construction of second-order...might be potassium niobate.) Because of this, the value of finding an "improved" material can be accurately gauged in a relative sense, and compared to
Pan, Shoukui; Okano, Y.; Tsunekawa, S.; Fukuda, T.
1993-03-01
The Kyropoulus method was used to grow nonlinear optical organic crystals ABP (4-aminobenzophenone). The crystals were characterized by nonlinear optical measurements and had a large effect of frequency doubling.
Nonlinear Quantum Optical Springs and Their Nonclassical Properties
International Nuclear Information System (INIS)
Faghihi, M.J.; Tavassoly, M.K.
2011-01-01
The original idea of quantum optical spring arises from the requirement of quantization of the frequency of oscillations in the Hamiltonian of harmonic oscillator. This purpose is achieved by considering a spring whose constant (and so its frequency) depends on the quantum states of another system. Recently, it is realized that by the assumption of frequency modulation of ω to ω√1+μa † a the mentioned idea can be established. In the present paper, we generalize the approach of quantum optical spring with particular attention to the dependence of frequency to the intensity of radiation field that naturally observes in the nonlinear coherent states, from which we arrive at a physical system has been called by us as nonlinear quantum optical spring. Then, after the introduction of the generalized Hamiltonian of nonlinear quantum optical spring and it's solution, we will investigate the nonclassical properties of the obtained states. Specially, typical collapse and revival in the distribution functions and squeezing parameters, as particular quantum features, will be revealed. (electromagnetism, optics, acoustics, heat transfer, classical mechanics, and fluid dynamics)
Nonlinear interaction of waves in an inhomogeneous plasma
International Nuclear Information System (INIS)
Istomin, Ya.N.
1988-01-01
Nonlinear wave processes in a weakly inhomogeneous plasma are considered. A quasilinear equation is derived which takes into account the effect of the waves on resonance particles, provided that the inhomogeneity appreciably affects the nature of the resonance interaction. Three-wave interaction is investigated under the same conditions. As an example, the nonlinear interaction in a relativistic plasma moving along a strong curvilinear magnetic field is considered
Optical nonlinear absorption characteristics of Sb2Se3 nanoparticles
Muralikrishna, Molli; Kiran, Aditha Sai; Ravikanth, B.; Sowmendran, P.; Muthukumar, V. Sai; Venkataramaniah, Kamisetti
2014-04-01
In this work, we report for the first time, the nonlinear optical absorption properties of antimony selenide (Sb2Se3) nanoparticles synthesized through solvothermal route. X-ray diffraction results revealed the crystalline nature of the nanoparticles. Electron microscopy studies revealed that the nanoparticles are in the range of 10 - 40 nm. Elemental analysis was performed using EDAX. By employing open aperture z-scan technique, we have evaluated the effective two-photon absorption coefficient of Sb2Se3 nanoparticles to be 5e-10 m/W at 532 nm. These nanoparticles exhibit strong intensity dependent nonlinear optical absorption and hence could be considered to have optical power limiting applications in the visible range.
Nonlinear Silicon Photonic Signal Processing Devices for Future Optical Networks
Directory of Open Access Journals (Sweden)
Cosimo Lacava
2017-01-01
Full Text Available In this paper, we present a review on silicon-based nonlinear devices for all optical nonlinear processing of complex telecommunication signals. We discuss some recent developments achieved by our research group, through extensive collaborations with academic partners across Europe, on optical signal processing using silicon-germanium and amorphous silicon based waveguides as well as novel materials such as silicon rich silicon nitride and tantalum pentoxide. We review the performance of four wave mixing wavelength conversion applied on complex signals such as Differential Phase Shift Keying (DPSK, Quadrature Phase Shift Keying (QPSK, 16-Quadrature Amplitude Modulation (QAM and 64-QAM that dramatically enhance the telecom signal spectral efficiency, paving the way to next generation terabit all-optical networks.
Macroscopic quantum effects in nonlinear optical patterns
International Nuclear Information System (INIS)
Gatti, A.; Lugiato, L.A.; Oppo, G.L.; Barnett, S.M.; Marzoli, I.
1998-01-01
We display the results of the numerical simulations of a set of Langevin equations, which describe the dynamics of a degenerate optical parametric oscillator in the Wigner representation. The scan of the threshold region shows the gradual transformation of a quantum image into a classical roll pattern. Thus the quantum image behaves as a precursor of the roll pattern which appear above threshold. In the fax field, suitable spatial correlation functions of intensity and field quadratures show unambiguously the quantum nature of fluctuations that generate the image, leading to effects of quantum noise reduction below the shot noise level and to the formulation of an EPR paradox. (author)
Optical computation based on nonlinear total reflectional optical ...
Indian Academy of Sciences (India)
2School of Education Science, South China Normal University, Guangzhou, 510631, China. *Corresponding ... Before the computation, all the inputs are prepared in the polarization state. The key .... The all-optical computing system described.
Nonlinear interactions of electromagnetic waves with the auroral ionosphere
Wong, Alfred Y.
1999-09-01
The ionosphere provides us with an opportunity to perform plasma experiments in an environment with long confinement times, very large-scale lengths, and no confining walls. The auroral ionosphere with its nearly vertical magnetic field geometry is uniquely endowed with large amount of free energy from electron and ion precipitation along the magnetic field and mega-ampere current across the magnetic field. To take advantage of this giant outdoor laboratory, two facilities HAARP and HIPAS, with frequencies ranging from the radio to optical bands, are now available for active probing of and interaction with this interesting region. The ponderomotive pressures from the self-consistent wave fields have produced significant local perturbations of density and particle distributions at heights where the incident EM frequency matches a plasma resonance. This paper will review theory and experiments covering the nonlinear phenomena of parametric decay instability to wave collapse processes. At HF frequencies plasma lenses can be created by preconditioning pulses to focus what is a normally divergent beam into a high-intensity spot to further enhance nonlinear phenomena. At optical wavelengths a large rotating liquid metal mirror is used to focus laser pulses up to a given height. Such laser pulses are tuned to the same wavelengths of selected atomic and molecular resonances, with resulting large scattering cross sections. Ongoing experiments on dual-site experiments and excitation of ELF waves will be presented. The connection of such basic studies to environmental applications will be discussed. Such applications include the global communication using ELF waves, the ozone depletion and remediation and the control of atmospheric CO2 through the use of ion cyclotron resonant heating.
Cross-Kerr nonlinearities in an optically dressed periodic medium
Energy Technology Data Exchange (ETDEWEB)
Slowik, K; Raczynski, A; Zaremba, J [Instytut Fizyki, Uniwersytet Mikolaja Kopernika, ulica Grudziadzka 5, 87-100 Torun (Poland); Zielinska-Kaniasty, S [Instytut Matematyki i Fizyki, Uniwersytet Technologiczno-Przyrodniczy, Aleja Prof. S Kaliskiego 7, 85-789 Bydgoszcz (Poland); Artoni, M [Department of Physics and Chemistry of Materials, CNR-INFM Sensor Lab, Brescia University and European Laboratory for Nonlinear Spectroscopy, Firenze (Italy); La Rocca, G C, E-mail: karolina@fizyka.umk.pl [Scuola Normale Superiore and CNISM, Pisa (Italy)
2011-02-15
Cross-Kerr nonlinearities are analyzed for two light beams propagating in an atomic medium in the tripod configuration, dressed by a strong standing-wave laser field that induces periodic optical properties. The reflection and transmission spectra as well as the phases of both the reflected and transmitted components of the two beams are analyzed theoretically with nonlinearities up to third order being taken into account. Ranges of parameters are sought in which the cross-Kerr effect can be used as the basis of the phase gate.
International Nuclear Information System (INIS)
Lorin, E; Bandrauk, A D; Lytova, M; Memarian, A
2015-01-01
This paper is dedicated to the exploration of non-conventional nonlinear optics models for intense and short electromagnetic fields propagating in a gas. When an intense field interacts with a gas, usual nonlinear optics models, such as cubic nonlinear Maxwell, wave and Schrödinger equations, derived by perturbation theory may become inaccurate or even irrelevant. As a consequence, and to include in particular the effect of free electrons generated by laser–molecule interaction, several heuristic models, such as UPPE, HOKE models, etc, coupled with Drude-like models [1, 2], were derived. The goal of this paper is to present alternative approaches based on non-heuristic principles. This work is in particular motivated by the on-going debate in the filamentation community, about the effect of high order nonlinearities versus plasma effects due to free electrons, in pulse defocusing occurring in laser filaments [3–9]. The motivation of our work goes beyond filamentation modeling, and is more generally related to the interaction of any external intense and (short) pulse with a gas. In this paper, two different strategies are developed. The first one is based on the derivation of an evolution equation on the polarization, in order to determine the response of the medium (polarization) subject to a short and intense electromagnetic field. Then, we derive a combined semi-heuristic model, based on Lewenstein’s strong field approximation model and the usual perturbative modeling in nonlinear optics. The proposed model allows for inclusion of high order nonlinearities as well as free electron plasma effects. (paper)
Nonlinear optics with coherent free electron lasers
Bencivenga, F.; Capotondi, F.; Mincigrucci, R.; Cucini, R.; Manfredda, M.; Pedersoli, E.; Principi, E.; Simoncig, A.; Masciovecchio, C.
2016-12-01
We interpreted the recent construction of free electron laser (FELs) facilities worldwide as an unprecedented opportunity to bring concepts and methods from the scientific community working with optical lasers into the domain of x-ray science. This motivated our efforts towards the realization of FEL-based wave-mixing applications. In this article we present new extreme ultraviolet transient grating (X-TG) data from vitreous SiO2, collected using two crossed FEL pulses (photon frequency 38 eV) to generate the X-TG and a phase matched optical probing pulse (photon frequency 3.1 eV). This experiment extends our previous investigation, which was carried out on a nominally identical sample using a different FEL photon frequency (45 eV) to excite the X-TG. The present data are featured by a peak intensity of the X-TG signal substantially larger than that previously reported and by slower modulations of the X-TG signal at positive delays. These differences could be ascribed to the different FEL photon energy used in the two experiments or to differences in the sample properties. A systematic X-TG study on the same sample as a function of the FEL wavelength is needed to draw a consistent conclusion. We also discuss how the advances in the performance of the FELs, in terms of generation of fully coherent photon pulses and multi-color FEL emission, may push the development of original experimental strategies to study matter at the femtosecond-nanometer time-length scales, with the unique option of element and chemical state specificity. This would allow the development of advanced experimental tools based on wave-mixing processes, which may have a tremendous impact in the study of a large array of phenomena, ranging from nano-dynamics in complex materials to charge and energy transfer processes.
DEFF Research Database (Denmark)
Guo, Hairun; Zeng, Xianglong; Zhou, Binbin
2013-01-01
We interpret the purely spectral forward Maxwell equation with up to third-order induced polarizations for pulse propagation and interactions in quadratic nonlinear crystals. The interpreted equation, also named the nonlinear wave equation in the frequency domain, includes quadratic and cubic...... nonlinearities, delayed Raman effects, and anisotropic nonlinearities. The full potential of this wave equation is demonstrated by investigating simulations of solitons generated in the process of ultrafast cascaded second-harmonic generation. We show that a balance in the soliton delay can be achieved due...
Report of workshop on X-ray and nonlinear optics
Energy Technology Data Exchange (ETDEWEB)
Nasu, Keiichiro; Namikawa, Kazumichi [eds.
1994-07-01
As synchrotron radiation has advanced to high luminance, the possibility of realizing coherent light has heightened, and the nonlinear optical phenomena in soft and hard X-ray regions have become the object of the concern of X-ray researchers, and also the researchers in the fields of quantum electronics and optical properties. This workshop was held on September 21 and 22, 1993 at National Laboratory for High energy Physics. Lectures were given on the generation of second harmonic of X-ray by utilizing dynamic diffraction, X-ray parametric scattering induced by strong laser beam, the resonance enhancement of X-ray inelastic scattering induced by strong visible light, Raman scattering in soft X-ray region, the control of nonlinear optical processes by strong external field; the experiments, though they are fundamental, they have not been carried out; undulator radiation X-ray and X-ray free electron laser, the improvement of the coherence of X-ray laser, superradiance of Frenkel excitor system and the measurement of superhigh speed pulses in X-ray region. The comment from the standpoint of the research on nonlinear optics was given. In this document, the gists of these lectures are collected. (K.I.).
Report of workshop on X-ray and nonlinear optics
International Nuclear Information System (INIS)
Nasu, Keiichiro; Namikawa, Kazumichi
1994-07-01
As synchrotron radiation has advanced to high luminance, the possibility of realizing coherent light has heightened, and the nonlinear optical phenomena in soft and hard X-ray regions have become the object of the concern of X-ray researchers, and also the researchers in the fields of quantum electronics and optical properties. This workshop was held on September 21 and 22, 1993 at National Laboratory for High energy Physics. Lectures were given on the generation of second harmonic of X-ray by utilizing dynamic diffraction, X-ray parametric scattering induced by strong laser beam, the resonance enhancement of X-ray inelastic scattering induced by strong visible light, Raman scattering in soft X-ray region, the control of nonlinear optical processes by strong external field; the experiments, though they are fundamental, they have not been carried out; undulator radiation X-ray and X-ray free electron laser, the improvement of the coherence of X-ray laser, superradiance of Frenkel excitor system and the measurement of superhigh speed pulses in X-ray region. The comment from the standpoint of the research on nonlinear optics was given. In this document, the gists of these lectures are collected. (K.I.)
Spin and diamagnetism in linear and nonlinear optics
International Nuclear Information System (INIS)
Andersen, Torsten; Keller, Ole; Huebner, Wolfgang; Johansson, Boerje
2004-01-01
We present a local-field theory for spin and diamagnetism in linear and nonlinear optics. We examine all the processes contained in the Pauli Hamiltonian and its corresponding microscopic current density, including the terms depending on the electron spin. The resulting general real-space conductivities are presented and discussed. To quantify the implications of including the spin, we study the linear and nonlinear optical properties of free-electron metals, represented by the screened homogeneous electron gas. The real-space formalism is transformed into Fourier space, and the symmetries of the linear and nonlinear optical conductivities in a homogeneous electron gas are discussed. Numerical results are presented for the homogeneous electron gas, in which we treat ω and q as independent variables, thereby opening the theory to near-field optics and the study of evanescent waves. We show that in regions of the ω-q spectrum, the presence of diamagnetism and spin dynamics significantly alters the response in comparison to considering only the paramagnetic response. Additionally, we discuss the effects of screening, and we finish our treatment by a discussion of how to connect the present theory to existing methods in ab initio solid-state physics
Ablation and optical third-order nonlinearities in Ag nanoparticles
Directory of Open Access Journals (Sweden)
Carlos Torres-Torres
2010-11-01
Full Text Available Carlos Torres-Torres1, Néstor Peréa-López2, Jorge Alejandro Reyes-Esqueda3, Luis Rodríguez-Fernández3, Alejandro Crespo-Sosa3, Juan Carlos Cheang-Wong3, Alicia Oliver31Section of Graduate Studies and Research, School of Mechanical and Electrical Engineering, National Polytechnic Institute, Zacatenco, Distrito Federal, Mexico; 2Laboratory for Nanoscience and Nanotechnology Research and Advanced Materials Department, IPICYT, Camino a la Presa San Jose, San Luis Potosi, Mexico; 3Instituto de Física, Universidad Nacional Autónoma de México, A.P. 20-364, México, D.F. 01000, MéxicoAbstract: The optical damage associated with high intensity laser excitation of silver nanoparticles (NPs was studied. In order to investigate the mechanisms of optical nonlinearity of a nanocomposite and their relation with its ablation threshold, a high-purity silica sample implanted with Ag ions was exposed to different nanosecond and picosecond laser irradiations. The magnitude and sign of picosecond refractive and absorptive nonlinearities were measured near and far from the surface plasmon resonance (SPR of the Ag NPs with a self-diffraction technique. Saturable optical absorption and electronic polarization related to self-focusing were identified. Linear absorption is the main process involved in nanosecond laser ablation, but nonlinearities are important for ultrashort picosecond pulses when the absorptive process become significantly dependent on the irradiance. We estimated that near the resonance, picosecond intraband transitions allow an expanded distribution of energy among the NPs, in comparison to the energy distribution resulting in a case of far from resonance, when the most important absorption takes place in silica. We measured important differences in the ablation threshold and we estimated that the high selectiveness of the SPR of Ag NPs as well as their corresponding optical nonlinearities can be strongly significant for laser
Self-similar optical pulses in competing cubic-quintic nonlinear media with distributed coefficients
International Nuclear Information System (INIS)
Zhang Jiefang; Tian Qing; Wang Yueyue; Dai Chaoqing; Wu Lei
2010-01-01
We present a systematic analysis of the self-similar propagation of optical pulses within the framework of the generalized cubic-quintic nonlinear Schroedinger equation with distributed coefficients. By appropriately choosing the relations between the distributed coefficients, we not only retrieve the exact self-similar solitonic solutions, but also find both the approximate self-similar Gaussian-Hermite solutions and compact solutions. Our analytical and numerical considerations reveal that proper choices of the distributed coefficients could make the unstable solitons stable and could restrict the nonlinear interaction between the neighboring solitons.
All-optical signal processing in quadratic nonlinear materials
DEFF Research Database (Denmark)
Johansen, Steffen Kjær
2002-01-01
of materials with a second order nonlinearity, the so-called X(2) materials, is faster and stronger than that of more conventional materials with a cubic nonlinearity. The X(2) materials support spatial solitons consisting of two coupled components, the fundamental wave (FW) and its second harmonic (SH......). During this project the interaction between such spatial solitons has been investigated theoretically through perturbation theory and experimentally via numerical simulations. The outcome of this research isnew theoretical tools for quantitatively predicting the escape angle, i.e. the angle of incidence...... are dedicated to this part of the research. In chapter 4 the generality of the theoretical approach is emphasised with the derivation and verification of equivalent tools for media with a saturable nonlinearity. The strength of the X(2) nonlinearity strongly depends on the phase mismatch between the FW...
Determination of optical constants and nonlinear optical coefficients ...
Indian Academy of Sciences (India)
of single crystals of organic molecules [12,13], organic molecules in a liquid solution. [14,15] and organic ... valence band 'tail states' might have a strong effect on the optical absorption resulting in ..... cm/W). The negative sign of the third-order.
ZnS/PVA nanocomposites for nonlinear optical applications
Ozga, K.; Michel, J.; Nechyporuk, B. D.; Ebothé, J.; Kityk, I. V.; Albassam, A. A.; El-Naggar, A. M.; Fedorchuk, A. O.
2016-07-01
We have found a correlation between ZnS nanocomposite nonlinear optical features and technological processing using electrolytic method. In the earlier researches this factor was neglected. However, it may open a new stage for operation by photovoltaic features of the well known semiconductors within a wide range of magnitudes. The titled nanostructured zinc sulfide (ZnS) was synthesized by electrolytic method. The obtained ZnS nano-crystallites possessed nano-particles sizes varying within 1.6 nm…1.8 nm. The titled samples were analyzed by XRD, HR-TEM, STEM, and nonlinear optical methods such as photo-induced two-photon absorption (TPA) and second harmonic generation (SHG). For this reason the nano-powders were embedded into the photopolymer poly(vinyl) alcohol (PVA) matrices. Role of aggregation in the mentioned properties is discussed. Possible origin of the such correlations are discussed.
Nonlinear optical polarization analysis in chemistry and biology
Simpson, Garth J
2017-01-01
This rigorous yet accessible guide presents a molecular-based description of nonlinear optical polarization analysis of chemical and biological assemblies. It includes discussion of the most common nonlinear optical microscopy and interfacial measurements used for quantitative analysis, specifically second harmonic generation (SHG), two-photon excited fluorescence (2PEF), vibrational sum frequency generation (SFG), and coherent anti-Stokes Raman spectroscopy/stimulated Raman spectroscopy (CARS/SRS). A linear algebra mathematical framework is developed, allowing step-wise systematic connections to be made between the observable measurements and the molecular response. Effects considered include local field corrections, the molecular orientation distribution, rotations between the molecular frame, the local frame and the laboratory frame, and simplifications from molecular and macromolecular symmetry. Specific examples are provided throughout the book, working from the common and relatively simple case studies ...
Dynamic nonlinear thermal optical effects in coupled ring resonators
Directory of Open Access Journals (Sweden)
Chenguang Huang
2012-09-01
Full Text Available We investigate the dynamic nonlinear thermal optical effects in a photonic system of two coupled ring resonators. A bus waveguide is used to couple light in and out of one of the coupled resonators. Based on the coupling from the bus to the resonator, the coupling between the resonators and the intrinsic loss of each individual resonator, the system transmission spectrum can be classified by three different categories: coupled-resonator-induced absorption, coupled-resonator-induced transparency and over coupled resonance splitting. Dynamic thermal optical effects due to linear absorption have been analyzed for each category as a function of the input power. The heat power in each resonator determines the thermal dynamics in this coupled resonator system. Multiple “shark fins” and power competition between resonators can be foreseen. Also, the nonlinear absorption induced thermal effects have been discussed.
International Nuclear Information System (INIS)
Li Biao; Chen Yong
2007-01-01
In this paper, the inhomogeneous nonlinear Schroedinger equation with the loss/gain and the frequency chirping is investigated. With the help of symbolic computation, three families of exact analytical solutions are presented by employing the extended projective Riccati equation method. From our results, many previous known results of nonlinear Schroedinger equation obtained by some authors can be recovered by means of some suitable selections of the arbitrary functions and arbitrary constants. Of optical and physical interests, soliton propagation and soliton interaction are discussed and simulated by computer, which include snake-soliton propagation and snake-solitons interaction, boomerang-like soliton propagation and boomerang-like solitons interaction, dispersion managed (DM) bright (dark) soliton propagation and DM solitons interaction
Symbolic computation of nonlinear wave interactions on MACSYMA
International Nuclear Information System (INIS)
Bers, A.; Kulp, J.L.; Karney, C.F.F.
1976-01-01
In this paper the use of a large symbolic computation system - MACSYMA - in determining approximate analytic expressions for the nonlinear coupling of waves in an anisotropic plasma is described. MACSYMA was used to implement the solutions of a fluid plasma model nonlinear partial differential equations by perturbation expansions and subsequent iterative analytic computations. By interacting with the details of the symbolic computation, the physical processes responsible for particular nonlinear wave interactions could be uncovered and appropriate approximations introduced so as to simplify the final analytic result. Details of the MACSYMA system and its use are discussed and illustrated. (Auth.)
Femtosecond nonlinear fiber optics in the ionization regime.
Hölzer, P; Chang, W; Travers, J C; Nazarkin, A; Nold, J; Joly, N Y; Saleh, M F; Biancalana, F; Russell, P St J
2011-11-11
By using a gas-filled kagome-style photonic crystal fiber, nonlinear fiber optics is studied in the regime of optically induced ionization. The fiber offers low anomalous dispersion over a broad bandwidth and low loss. Sequences of blueshifted pulses are emitted when 65 fs, few-microjoule pulses, corresponding to high-order solitons, are launched into the fiber and undergo self-compression. The experimental results are confirmed by numerical simulations which suggest that free-electron densities of ∼10(17) cm(-3) are achieved at peak intensities of 10(14) W/cm(2) over length scales of several centimeters.
Signaling on the continuous spectrum of nonlinear optical fiber.
Tavakkolnia, Iman; Safari, Majid
2017-08-07
This paper studies different signaling techniques on the continuous spectrum (CS) of nonlinear optical fiber defined by nonlinear Fourier transform. Three different signaling techniques are proposed and analyzed based on the statistics of the noise added to CS after propagation along the nonlinear optical fiber. The proposed methods are compared in terms of error performance, distance reach, and complexity. Furthermore, the effect of chromatic dispersion on the data rate and noise in nonlinear spectral domain is investigated. It is demonstrated that, for a given sequence of CS symbols, an optimal bandwidth (or symbol rate) can be determined so that the temporal duration of the propagated signal at the end of the fiber is minimized. In effect, the required guard interval between the subsequently transmitted data packets in time is minimized and the effective data rate is significantly enhanced. Moreover, by selecting the proper signaling method and design criteria a distance reach of 7100 km is reported by only singling on CS at a rate of 9.6 Gbps.
Structure, Electronic and Nonlinear Optical Properties of Furyloxazoles and Thienyloxazoles
International Nuclear Information System (INIS)
Dagli, Ozlem; Gok, Rabia; Bahat, Mehmet; Ozbay, Akif
2016-01-01
Geometry optimization, electronic and nonlinear optical properties of isomers of furyloxazole and thienyloxazole molecules are carried out at the B3LYP/6-311++G(2d,p) level. The conformational analysis of 12 compounds have been studied as a function of torsional angle between rings. Electronic and NLO properties such as dipole moment, energy gap, polarizability and first hyperpolarizability were also calculated. (paper)
Optically nonlinear energy transfer in light-harvesting dendrimers
Andrews, David; Bradshaw, DS
2004-01-01
Dendrimeric polymers are the subject of intense research activity geared towards their implementation in nanodevice applications such as energy harvesting systems,organic light-emitting diodes, photosensitizers, low-threshold lasers, and quantum logic elements, etc. A recent development in this area has been the construction of dendrimers specifically designed to exhibit novel forms of optical nonlinearity, exploiting the unique properties of these materials at high levels of photon flux. Sta...
International Nuclear Information System (INIS)
Arie, A.
1999-01-01
Nonlinear frequency mixing processes, e.g. second harmonic generation, sum and difference frequency generation, etc., require matching of the phases of the interacting waves. The traditional method to achieve it is by selecting a specific angle of propagation in a birefringent nonlinear crystal. The main limitation of the birefringent phase matching method stems from the fact that for many interesting interactions, the phase matching condition cannot be satisfied in a specific crystal. This obstacle can be removed by the technique of quasi-phase-matching (QPM), where the nonlinear coefficient of the material is modulated at a fixed spatial frequency that equals the wave-vector phase mismatch between the interacting waves. An important development in recent years is the ability to periodically reverse the sign of the nonlinear coefficient in ferroelectric crystals by applying a high electric field through a periodic electrode. Some recent QPM interactions in periodically-poled KTP that were recently achieved at Tel-Aviv University include continuous-wave optical parametric oscillations, as well as generation of tunable mid-infrared radiation by difference frequency generation. Periodic patterning of the nonlinear coefficient enables to phase match only a single interaction. It would be advantageous to further extend the applications of this technique in order to simultaneously satisfy several interactions on a single crystal. This cannot be usually achieved in a periodic pattern, however more sophisticated quasi-periodic structures can be designed in this case. An interesting analogy can be drawn between artificially-made quasi-periodically-patterned nonlinear crystals and quasi-crystals found in nature, in rapidly-cooled metallic alloys
Nonlinear optical and electroabsorption spectra of polydiacetylene crystals and films
Mukhopadhyay, D.; Soos, Z. G.
1996-01-01
Vibronic structure of nonlinear optical (NLO) coefficients is developed within the Condon approximation, displaced harmonic oscillators, and crude adiabatic states. The displacements of backbone modes of conjugated polymers are taken from vibrational data on the ground and 1B excited state. NLO resonances are modeled by three excitations and transition moments taken from Pariser-Parr-Pople (PPP) theory and optimized to polydiacetylene (PDA) spectra in crystals and films, with blue-shifted 1B exciton. The joint analysis of third-harmonic-generation, two-photon absorption, and nondegenerate four-wave-mixing spectra of PDA crystals and films shows weak two-photon absorption to 2A below 1B, leading to overlapping resonances in the THG spectrum, strong two-photon absorption to an nA state some 35% above 1B, and weak Raman resonances in nondegenerate FWM spectra. The full π-π* spectrum contributes to Stark shifts and field-induced transitions, as shown by PPP results for PDA oligomers. The Stark shift dominates high-resolution electroabsorption (EA) spectra of PDA crystals below 10 K. The close correspondence between EA and the first-derivative I'(ω) of the linear absorption above the 1B exciton in PDA crystals provides an experimental separation of vibrational and electronic contributions that limits any even-parity state in this 0.5 eV interval. An oscillator-strength sum rule is applied to the convergence of PDA oligomers with increasing length, N, and the crystal oscillator strengths are obtained without adjustable parameters. The sum rule for the 1B exciton implies large transition moments to higher-energy Ag states, whose locations in recent models are contrasted to PPP results. Joint analysis of NLO and EA spectra clarifies when a few electronic excitations are sufficient, distinguishes between vibrational and electronic contributions, and supports similar π-electron interactions in conjugated molecules and polymers.
Dye-Induced Enhancement of Optical Nonlinearity in Liquids and Liquid Crystals
International Nuclear Information System (INIS)
Muenster, R.; Jarasch, M.; Zhuang, X.; Shen, Y.
1997-01-01
Optical nonlinearity of liquid crystals (LC) in the isotropic phase can be enhanced by 1 order of magnitude by dissolving 0.1% of anthraquinone dye in the LC. The enhancement decreases by ∼30% when the LC transforms into the nematic phase. The same guest-host effect also exists in non-LC liquids. It can be explained by a model based on the change of guest-host interaction induced by optical excitations of the dye. copyright 1996 The American Physical Society
Optical rogue waves generation in a nonlinear metamaterial
Onana Essama, Bedel Giscard; Atangana, Jacques; Biya-Motto, Frederick; Mokhtari, Bouchra; Cherkaoui Eddeqaqi, Noureddine; Kofane, Timoleon Crepin
2014-11-01
We investigate the behavior of electromagnetic wave which propagates in a metamaterial for negative index regime. The optical pulse propagation is described by the nonlinear Schrödinger equation with cubic-quintic nonlinearities, second- and third-order dispersion effects. The behavior obtained for negative index regime is compared to that observed for positive index regime. The characterization of electromagnetic wave uses some pulse parameters obtained analytically and called collective coordinates such as amplitude, temporal position, width, chirp, frequency shift and phase. Six frequency ranges have been pointed out where a numerical evolution of collective coordinates and their stability are studied under a typical example to verify our analysis. It appears that a robust soliton due to a perfect compensation process between second-order dispersion and cubic-nonlinearity is presented at each frequency range for both negative and positive index regimes. Thereafter, the stability of the soliton pulse and physical conditions leading to optical rogue waves generation are discussed at each frequency range for both regimes, when third-order dispersion and quintic-nonlinearity come into play. We have demonstrated that collective coordinates give much useful information on external and internal behavior of rogue events. Firstly, we determine at what distance begins the internal excitation leading to rogue waves. Secondly, what kind of internal modification and how it modifies the system in order to build-up rogue events. These results lead to a best comprehension of the mechanism of rogue waves generation. So, it clearly appears that the rogue wave behavior strongly depends on nonlinearity strength of distortion, frequency and regime considered.
Gallium nitride on gallium oxide substrate for integrated nonlinear optics
Awan, Kashif M.; Dolgaleva, Ksenia; Mumthaz Muhammed, Mufasila; Roqan, Iman S.
2017-01-01
Gallium Nitride (GaN), being a direct bandgap semiconductor with a wide bandgap and high thermal stability, is attractive for optoelectronic and electronic applications. Furthermore, due to its high optical nonlinearity — the characteristic of all 111-V semiconductors — GaN is also expected to be a suitable candidate for integrated nonlinear photonic circuits for a plethora of apphcations, ranging from on-chip wavelength conversion to quantum computing. Although GaN devices are in commercial production, it still suffers from lack of a suitable substrate material to reduce structural defects like high densities of threading dislocations (TDs), stacking faults, and grain boundaries. These defects significandy deteriorate the optical quality of the epi-grown GaN layer, since they act as non-radiative recombination centers. Recent studies have shown that GaN grown on (−201) β-Gallium Oxide (Ga
Polycarbonate-Based Blends for Optical Non-linear Applications
Stanculescu, F.; Stanculescu, A.
2016-02-01
This paper presents some investigations on the optical and morphological properties of the polymer (matrix):monomer (inclusion) composite materials obtained from blends of bisphenol A polycarbonate and amidic monomers. For the preparation of the composite films, we have selected monomers characterised by a maleamic acid structure and synthesised them starting from maleic anhydride and aniline derivatives with -COOH, -NO2, -N(C2H5)2 functional groups attached to the benzene ring. The composite films have been deposited by spin coating using a mixture of two solutions, one containing the matrix and the other the inclusion, both components of the composite system being dissolved in the same solvent. The optical transmission and photoluminescence properties of the composite films have been investigated in correlation with the morphology of the films. The scanning electron microscopy and atomic force microscopy have revealed a non-uniform morphology characterised by the development of two distinct phases. We have also investigated the generation of some optical non-linear (ONL) phenomena in these composite systems. The composite films containing as inclusions monomers characterised by the presence of one -COOH or two -NO2 substituent groups to the aromatic nucleus have shown the most intense second-harmonic generation (SHG). The second-order optical non-linear coefficients have been evaluated for these films, and the effect of the laser power on the ONL behaviour of these materials has also been emphasised.
Nonlinear optical characteristics of monolayer MoSe{sub 2}
Energy Technology Data Exchange (ETDEWEB)
Le, Chinh Tam; Ullah, Farman; Senthilkumar, Velusamy; Kim, Yong Soo [Department of Physics and Energy Harvest Storage Research Center, University of Ulsan (Korea, Republic of); Clark, Daniel J.; Jang, Joon I. [Department of Physics, Applied Physics and Astronomy, Binghamton University, Binghamton, NY (United States); Sim, Yumin; Seong, Maeng-Je [Department of Physics, Chung-Ang University, Seoul (Korea, Republic of); Chung, Koo-Hyun [School of Mechanical Engineering, University of Ulsan (Korea, Republic of); Park, Hyoyeol [Electronics, Communication and Semiconductor Applications Department, Ulsan College (Korea, Republic of)
2016-08-15
In this study, we utilized picosecond pulses from an Nd:YAG laser to investigate the nonlinear optical characteristics of monolayer MoSe{sub 2}. Two-step growth involving the selenization of pulsed-laser-deposited MoO{sub 3} film was employed to yield the MoSe{sub 2} monolayer on a SiO{sub 2}/Si substrate. Raman scattering, photoluminescence (PL) spectroscopy, and atomic force microscopy verified the high optical quality of the monolayer. The second-order susceptibility χ{sup (2)} was calculated to be ∝50 pm V{sup -1} at the second harmonic wavelength λ{sub SHG} ∝810 nm, which is near the optical gap of the monolayer. Interestingly, our wavelength-dependent second harmonic scan can identify the bound excitonic states including negatively charged excitons much more efficiently, compared with the PL method at room temperature. Additionally, the MoSe{sub 2} monolayer exhibits a strong laser-induced damage threshold ∝16 GW cm{sup -2} under picosecond-pulse excitation{sub .} Our findings suggest that monolayer MoSe{sub 2} can be considered as a promising candidate for high-power, thin-film-based nonlinear optical devices and applications. (copyright 2016 by WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)
Gallium nitride on gallium oxide substrate for integrated nonlinear optics
Awan, Kashif M.
2017-11-22
Gallium Nitride (GaN), being a direct bandgap semiconductor with a wide bandgap and high thermal stability, is attractive for optoelectronic and electronic applications. Furthermore, due to its high optical nonlinearity — the characteristic of all 111-V semiconductors — GaN is also expected to be a suitable candidate for integrated nonlinear photonic circuits for a plethora of apphcations, ranging from on-chip wavelength conversion to quantum computing. Although GaN devices are in commercial production, it still suffers from lack of a suitable substrate material to reduce structural defects like high densities of threading dislocations (TDs), stacking faults, and grain boundaries. These defects significandy deteriorate the optical quality of the epi-grown GaN layer, since they act as non-radiative recombination centers. Recent studies have shown that GaN grown on (−201) β-Gallium Oxide (Ga
Progress Toward Single-Photon-Level Nonlinear Optics in Crystalline Microcavities
Kowligy, Abijith S.
Over the last two decades, the emergence of quantum information science has uncovered many practical applications in areas such as communications, imaging, and sensing where harnessing quantum features of Nature provides tremendous benefits over existing methods exploiting classical physical phenomena. In this effort, one of the frontiers of research has been to identify and utilize quantum phenomena that are not susceptible to environmental and parasitic noise processes. Quantum photonics has been at the forefront of these studies because it allows room-temperature access to its inherently quantum-mechanical features, and allows leveraging the mature telecommunication industry. Accompanying the weak environmental influence, however, are also weak optical nonlinearities. Efficient nonlinear optical interactions are indispensible for many of the existing protocols for quantum optical computation and communication, e.g. high-fidelity entangling quantum logic gates rely on large nonlinear responses at the one- or few-photon-level. While this has been addressed to a great extent by interfacing photons with single quantum emitters and cold atomic gases, scalability has remained elusive. In this work, we identify the macroscopic second-order nonlinear polarization as a robust platform to address this challenge, and utilize the recent advances in the burgeoning field of optical microcavities to enhance this nonlinear response. In particular, we show theoretically that by using the quantum Zeno effect, low-noise, single-photon-level optical nonlinearities can be realized in lithium niobate whispering-gallery-mode microcavities, and present experimental progress toward this goal. Using the measured strength of the second-order nonlinear response in lithium niobate, we modeled the nonlinear system in the strong coupling regime using the Schrodinger picture framework and theoretically demonstrated that the single-photon-level operation can be observed for cavity lifetimes in
Nonlinear optical activity in Bridgman growth layered compounds
Energy Technology Data Exchange (ETDEWEB)
Miah, M.I., E-mail: m.miah@griffith.edu.au [Queensland Micro- and Nanotechnology Centre, Griffith University, Nathan, Brisbane, QLD 4111 (Australia); Biomolecular and Physical Sciences, Griffith University, Nathan, Brisbane, QLD 4111 (Australia); Department of Physics, University of Chittagong, Chittagong 4331 (Bangladesh)
2010-02-15
Layered semiconductor compound CdI{sub 2} has been grown with the Bridgman technique and studied by nonlinear transmittance spectroscopy. The optical absorption in CdI{sub 2} shows a nonlinear transmission of the incident laser power (P{sub 0}) within a lower power limit. The transmission, however, is found to saturate at high powers, giving a clamped output. The value of the incident power (P{sub 0C}) at which clamping starts is also found to depend on the crystal temperature (T{sub L}). The values of P{sub OC} ranges from 55 to 65 MW cm{sup -2} for T{sub L} = 4.2-180 K. The dynamic range (D{sub R}) as a function of T{sub L} is calculated and the values are found to range from D{sub R} = 2 to 1.6. The optical limiting mechanisms are discussed. The two-photon absorption (TPA) coefficient ({beta}) of the optical nonlinear process in CdI{sub 2} is estimated. The values are found to be within a range from {beta} = 47 to 25 cm GW{sup -1} and be decreasing with increasing T{sub L}. As expected for the TPA process, the experimental data within a certain range follows the linear relation: log (P{sub 0}/P{sub T}) = A{sub G} + {Omega}(P{sub 0} - P{sub T}), where P{sub T} is the transmitted power, A{sub G} is the absorbance of the ground state and {Omega} is a constant depending on the absorption cross-section and the relaxation time. The values of A{sub G} and {Omega} estimated from the fits to the measured data vary with T{sub L}. The findings resulting from this investigation might have potential applications in optical sensors protection.
Nonlinear optical response and its theoretical modelling of Sb2S3 nanorod
Yadav, Rajesh Kumar; Barik, A. R.; Das, Amlan; Adarsh, K. V.
2018-05-01
Light-matter interaction in nanoscale regime have unprecedented and accelerating demand in optoelectronics, valley electronics and device applications. Such interaction in 1-dimention (1D) metal chalcogenides has emerged as an important research topic because of its possibility to custom design optical properties, implying enormous application including optical computers, communications, bioimaging, and so on. However, understanding of nonlinear optical response of these nanostructures is still lacking, although it constitutes an interesting problem on the light-matter interaction. Here, we have presented the nonlinear optical response in Sb2S3 nanorod using Z-scan technique. Our experimental findings show a strong saturable absorption (SA). In this context, we have numerically simulated the experimental result using two level rate equation. The solutions of these two-level rate equation for a Gaussian shaped pulse exactly replicated the experimental data. From the best numerical fit, we found excited state decay time (τ ≈ 0.15ns) and saturation intensity (IS ≈ 0.01 GW/cm2). Additionally, we have calculated number of career density (N ≈ 5.31 × 10-17 cm-3), ground state absorption cross section (σ1 ≈ 1.63 × 10-17 cm2). Our experimental finding indicates that they can be employed as saturable absorbers.
Spatial optical (2+1)-dimensional scalar- and vector-solitons in saturable nonlinear media
Energy Technology Data Exchange (ETDEWEB)
Weilnau, C.; Traeger, D.; Schroeder, J.; Denz, C. [Institute of Applied Physics, Westfaelische Wilhelms-Universitaet Muenster, Corrensstr. 2/4, 48149 Muenster (Germany); Ahles, M.; Petter, J. [Institute of Applied Physics, Technische Universitaet Darmstadt, Hochschulstr. 6, 64289 Darmstadt (Germany)
2002-10-01
(2+1)-dimensional optical spatial solitons have become a major field of research in nonlinear physics throughout the last decade due to their potential in adaptive optical communication technologies. With the help of photorefractive crystals that supply the required type of nonlinearity for soliton generation, we are able to demonstrate experimentally the formation, the dynamic properties, and especially the interaction of solitary waves, which were so far only known from general soliton theory. Among the complex interaction scenarios of scalar solitons, we reveal a distinct behavior denoted as anomalous interaction, which is unique in soliton-supporting systems. Further on, we realize highly parallel, light-induced waveguide configurations based on photorefractive screening solitons that give rise to technical applications towards waveguide couplers and dividers as well as all-optical information processing devices where light is controlled by light itself. Finally, we demonstrate the generation, stability and propagation dynamics of multi-component or vector solitons, multipole transverse optical structures bearing a complex geometry. In analogy to the particle-light dualism of scalar solitons, various types of vector solitons can - in a broader sense - be interpreted as molecules of light. (Abstract Copyright [2002], Wiley Periodicals, Inc.)
Spatial optical (2+1)-dimensional scalar- and vector-solitons in saturable nonlinear media
International Nuclear Information System (INIS)
Weilnau, C.; Traeger, D.; Schroeder, J.; Denz, C.; Ahles, M.; Petter, J.
2002-01-01
(2+1)-dimensional optical spatial solitons have become a major field of research in nonlinear physics throughout the last decade due to their potential in adaptive optical communication technologies. With the help of photorefractive crystals that supply the required type of nonlinearity for soliton generation, we are able to demonstrate experimentally the formation, the dynamic properties, and especially the interaction of solitary waves, which were so far only known from general soliton theory. Among the complex interaction scenarios of scalar solitons, we reveal a distinct behavior denoted as anomalous interaction, which is unique in soliton-supporting systems. Further on, we realize highly parallel, light-induced waveguide configurations based on photorefractive screening solitons that give rise to technical applications towards waveguide couplers and dividers as well as all-optical information processing devices where light is controlled by light itself. Finally, we demonstrate the generation, stability and propagation dynamics of multi-component or vector solitons, multipole transverse optical structures bearing a complex geometry. In analogy to the particle-light dualism of scalar solitons, various types of vector solitons can - in a broader sense - be interpreted as molecules of light. (Abstract Copyright [2002], Wiley Periodicals, Inc.)
Nonclassical properties of a contradirectional nonlinear optical coupler
Energy Technology Data Exchange (ETDEWEB)
Thapliyal, Kishore [Jaypee Institute of Information Technology, A-10, Sector-62, Noida, UP-201307 (India); Pathak, Anirban, E-mail: anirban.pathak@gmail.com [Jaypee Institute of Information Technology, A-10, Sector-62, Noida, UP-201307 (India); RCPTM, Joint Laboratory of Optics of Palacky University and Institute of Physics of Academy of Science of the Czech Republic, Faculty of Science, Palacky University, 17. listopadu 12, 771 46 Olomouc (Czech Republic); Sen, Biswajit [Department of Physics, Vidyasagar Teachers' Training College, Midnapore 721101 (India); Perřina, Jan [RCPTM, Joint Laboratory of Optics of Palacky University and Institute of Physics of Academy of Science of the Czech Republic, Faculty of Science, Palacky University, 17. listopadu 12, 771 46 Olomouc (Czech Republic); Department of Optics, Palacky University, 17. listopadu 12, 771 46 Olomouc (Czech Republic)
2014-10-24
We investigate the nonclassical properties of output fields propagated through a contradirectional asymmetric nonlinear optical coupler consisting of a linear waveguide and a nonlinear (quadratic) waveguide operated by second harmonic generation. In contrast to the earlier results, all the initial fields are considered weak and a completely quantum-mechanical model is used here to describe the system. Perturbative solutions of Heisenberg's equations of motion for various field modes are obtained using Sen–Mandal technique. Obtained solutions are subsequently used to show the existence of single-mode and intermodal squeezing, single-mode and intermodal antibunching, two-mode and multi-mode entanglement in the output of contradirectional asymmetric nonlinear optical coupler. Further, existence of higher order nonclassicality is also established by showing the existence of higher order antibunching, higher order squeezing and higher order entanglement. Variation of observed nonclassical characters with different coupling constants and phase mismatch is discussed. - Highlights: • Nonclassicalities in fields propagating through a directional coupler is studied. • Completely quantum-mechanical description of the coupler is provided. • Analytic solutions of Heisenberg equations of motion for various modes are obtained. • Existence of lower order and higher order entanglement is shown. • Variation of nonclassicalities with phase-mismatch and coupling constants is studied.
Semiclassical Path Integral Calculation of Nonlinear Optical Spectroscopy.
Provazza, Justin; Segatta, Francesco; Garavelli, Marco; Coker, David F
2018-02-13
Computation of nonlinear optical response functions allows for an in-depth connection between theory and experiment. Experimentally recorded spectra provide a high density of information, but to objectively disentangle overlapping signals and to reach a detailed and reliable understanding of the system dynamics, measurements must be integrated with theoretical approaches. Here, we present a new, highly accurate and efficient trajectory-based semiclassical path integral method for computing higher order nonlinear optical response functions for non-Markovian open quantum systems. The approach is, in principle, applicable to general Hamiltonians and does not require any restrictions on the form of the intrasystem or system-bath couplings. This method is systematically improvable and is shown to be valid in parameter regimes where perturbation theory-based methods qualitatively breakdown. As a test of the methodology presented here, we study a system-bath model for a coupled dimer for which we compare against numerically exact results and standard approximate perturbation theory-based calculations. Additionally, we study a monomer with discrete vibronic states that serves as the starting point for future investigation of vibronic signatures in nonlinear electronic spectroscopy.
Time-resolved analysis of nonlinear optical limiting for laser synthesized carbon nanoparticles
Chen, G. X.; Hong, M. H.
2010-11-01
Nonlinear optical limiting materials have attracted much research interest in recent years. Carbon nanoparticles suspended in liquids show a strong nonlinear optical limiting function. It is important to investigate the nonlinear optical limiting process of carbon nanoparticles for further improving their nonlinear optical limiting performance. In this study, carbon nanoparticles were prepared by laser ablation of a carbon target in tetrahydrofuran (THF). Optical limiting properties of the samples were studied with 532-nm laser light, which is in the most sensitive wavelength band for human eyes. The shape of the laser pulse plays an important role for initializing the nonlinear optical limiting effect. Time-resolved analysis of laser pulses discovered 3 fluence stages of optical limiting. Theoretical simulation indicates that the optical limiting is initialized by a near-field optical enhancement effect.
Nonlinear light scattering in a two component medium: optical limiting application
International Nuclear Information System (INIS)
Joudrier, Valerie
1998-01-01
Scattering is a fundamental manifestation of the interaction between matter and radiation, resulting from inhomogeneities in the refractive index, which decrease transmission. This phenomenon is then especially attractive for sensor protection from laser light by optical limiting. One of the methods to induce scattering at high incident energy is to make use of the Kerr effect where the index of refraction is intensity dependent. Thus, the idea is to use a two component medium with a good index matching between the two components at low intensity, resulting in the medium transparency, and to modify it, at high intensity, due to the non linearity of one component making the medium highly scattering. Some of the experimental and theoretical investigations concerning a new material (here, a cell containing some liquid with small silica particles as inclusion in it) are presented in the visible domain (I=532 nm), for the nanosecond protection regime, beginning, with the chemical synthesis of the sample. The experimental results concerning the optical limiting process are presented, showing that nonlinear scattering is clearly the dominant mechanism in confrontation with other potential nonlinear effects. Several complementary experiments are then performed to complete the nonlinear scattering characterization, involving the measurement of the angular distribution of scattered energy and the integrating sphere measurement. Further information are also gained by studying the time response of the nonlinearities with a dual-beam (pulsed-pump, cw probe) technique. The previous experimental data is also analyzed with some simple theoretical models to evaluate the nonlinearity of the material from optical limiting, the angular scattering and the total scattering energy measurements. The good match between all the analytical results permits to delineate the physical mechanisms responsible for the nonlinear scattering effect and to direct the final conclusion. (author) [fr
Inference of a Nonlinear Stochastic Model of the Cardiorespiratory Interaction
Smelyanskiy, V. N.; Luchinsky, D. G.; Stefanovska, A.; McClintock, P. V.
2005-03-01
We reconstruct a nonlinear stochastic model of the cardiorespiratory interaction in terms of a set of polynomial basis functions representing the nonlinear force governing system oscillations. The strength and direction of coupling and noise intensity are simultaneously inferred from a univariate blood pressure signal. Our new inference technique does not require extensive global optimization, and it is applicable to a wide range of complex dynamical systems subject to noise.
Nonlinear PCA: characterizing interactions between modes of brain activity.
Friston, K; Phillips, J; Chawla, D; Büchel, C
2000-01-01
This paper presents a nonlinear principal component analysis (PCA) that identifies underlying sources causing the expression of spatial modes or patterns of activity in neuroimaging time-series. The critical aspect of this technique is that, in relation to conventional PCA, the sources can interact to produce (second-order) spatial modes that represent the modulation of one (first-order) spatial mode by another. This nonlinear PCA uses a simple neural network architecture that embodies a spec...
Matter-wave two-dimensional solitons in crossed linear and nonlinear optical lattices
International Nuclear Information System (INIS)
Luz, H. L. F. da; Gammal, A.; Abdullaev, F. Kh.; Salerno, M.; Tomio, Lauro
2010-01-01
The existence of multidimensional matter-wave solitons in a crossed optical lattice (OL) with a linear optical lattice (LOL) in the x direction and a nonlinear optical lattice (NOL) in the y direction, where the NOL can be generated by a periodic spatial modulation of the scattering length using an optically induced Feshbach resonance is demonstrated. In particular, we show that such crossed LOLs and NOLs allow for stabilizing two-dimensional solitons against decay or collapse for both attractive and repulsive interactions. The solutions for the soliton stability are investigated analytically, by using a multi-Gaussian variational approach, with the Vakhitov-Kolokolov necessary criterion for stability; and numerically, by using the relaxation method and direct numerical time integrations of the Gross-Pitaevskii equation. Very good agreement of the results corresponding to both treatments is observed.
Matter-wave two-dimensional solitons in crossed linear and nonlinear optical lattices
da Luz, H. L. F.; Abdullaev, F. Kh.; Gammal, A.; Salerno, M.; Tomio, Lauro
2010-10-01
The existence of multidimensional matter-wave solitons in a crossed optical lattice (OL) with a linear optical lattice (LOL) in the x direction and a nonlinear optical lattice (NOL) in the y direction, where the NOL can be generated by a periodic spatial modulation of the scattering length using an optically induced Feshbach resonance is demonstrated. In particular, we show that such crossed LOLs and NOLs allow for stabilizing two-dimensional solitons against decay or collapse for both attractive and repulsive interactions. The solutions for the soliton stability are investigated analytically, by using a multi-Gaussian variational approach, with the Vakhitov-Kolokolov necessary criterion for stability; and numerically, by using the relaxation method and direct numerical time integrations of the Gross-Pitaevskii equation. Very good agreement of the results corresponding to both treatments is observed.
Vibrational spectroscopic and non-linear optical activity studies on nicotinanilide : A DFT approach
Premkumar, S.; Jawahar, A.; Mathavan, T.; Dhas, M. Kumara; Benial, A. Milton Franklin
2015-06-01
The molecular structure of nicotinanilide was optimized by the DFT/B3LYP method with cc-pVTZ basis set using Gaussian 09 program. The first order hyperpolarizability of the molecule was calculated, which exhibits the higher nonlinear optical activity. The natural bond orbital analysis confirms the presence of intramolecular charge transfer and the hydrogen bonding interaction, which leads to the higher nonlinear optical activity of the molecule. The Frontier molecular orbitals analysis of the molecule shows that the delocalization of electron density occurs within the molecule. The lower energy gap indicates that the hydrogen bond formation between the charged species. The vibrational frequencies were calculated and assigned on the basis of potential energy distribution calculation using the VEDA 4.0 program and the corresponding vibrational spectra were simulated. Hence, the nicotinanilide molecule can be a good candidate for second-order NLO material.
Nonlinear optical properties of colloidal silver nanoparticles produced by laser ablation in liquids
International Nuclear Information System (INIS)
Karavanskii, V A; Krasovskii, V I; Ivanchenko, P V; Simakin, Aleksandr V
2004-01-01
The optical and nonlinear optical properties of colloidal solutions of silver obtained by laser ablation in water and ethanol are studied. It is shown that freshly prepared colloids experience a full or partial sedimentation by changing their nonlinear optical properties. Aqueous colloids undergo a partial sedimentation and their nonlinear optical absorption changes to nonlinear optical transmission. The obtained results are interpreted using the Drude model for metal particles taking the particle size into account and can be explained by the sedimentation of larger silver particles accompanied by the formation of a stable colloid containing silver nanoparticles with a tentatively silver oxide shell. The characteristic size of particles forming such a stable colloid is determined and its optical nonlinearity is estimated. (nonlinear optical phenomena)
Assessment of fibrotic liver disease with multimodal nonlinear optical microscopy
Lu, Fake; Zheng, Wei; Tai, Dean C. S.; Lin, Jian; Yu, Hanry; Huang, Zhiwei
2010-02-01
Liver fibrosis is the excessive accumulation of extracellular matrix proteins such as collagens, which may result in cirrhosis, liver failure, and portal hypertension. In this study, we apply a multimodal nonlinear optical microscopy platform developed to investigate the fibrotic liver diseases in rat models established by performing bile duct ligation (BDL) surgery. The three nonlinear microscopy imaging modalities are implemented on the same sectioned tissues of diseased model sequentially: i.e., second harmonic generation (SHG) imaging quantifies the contents of the collagens, the two-photon excitation fluorescence (TPEF) imaging reveals the morphology of hepatic cells, while coherent anti-Stokes Raman scattering (CARS) imaging maps the distributions of fats or lipids quantitatively across the tissue. Our imaging results show that during the development of liver fibrosis (collagens) in BDL model, fatty liver disease also occurs. The aggregated concentrations of collagen and fat constituents in liver fibrosis model show a certain correlationship between each other.
Higher-order modulation instability in nonlinear fiber optics.
Erkintalo, Miro; Hammani, Kamal; Kibler, Bertrand; Finot, Christophe; Akhmediev, Nail; Dudley, John M; Genty, Goëry
2011-12-16
We report theoretical, numerical, and experimental studies of higher-order modulation instability in the focusing nonlinear Schrödinger equation. This higher-order instability arises from the nonlinear superposition of elementary instabilities, associated with initial single breather evolution followed by a regime of complex, yet deterministic, pulse splitting. We analytically describe the process using the Darboux transformation and compare with experiments in optical fiber. We show how a suitably low frequency modulation on a continuous wave field induces higher-order modulation instability splitting with the pulse characteristics at different phases of evolution related by a simple scaling relationship. We anticipate that similar processes are likely to be observed in many other systems including plasmas, Bose-Einstein condensates, and deep water waves. © 2011 American Physical Society
Fractals: Giant impurity nonlinearities in optics of fractal clusters
International Nuclear Information System (INIS)
Butenko, A.V.; Shalaev, V.M.; Stockman, M.I.
1988-01-01
A theory of nonlinear optical properties of fractals is developed. Giant enhancement of optical susceptibilities is predicted for impurities bound to a fractal. This enhancement occurs if the exciting radiation frequency lies within the absorption band of the fractal. The giant optical nonlinearities are due to existence of high local electric fields in the sites of impurity locations. Such fields are due to the inhomogeneously broadened character of a fractal spectrum, i.e. partial conservation of individuality of fractal-forming particles (monomers). The field enhancement is proportional to the Q-factor of the resonance of a monomer. The effects of coherent anti-Stokes Raman scattering (CARS) and phase conjugation (PC) of light waves are enhanced to a much greater degree than generation of higher harmonics. In a general case the susceptibility of a higher-order is enhanced in the maximum way if the process includes ''subtraction'' of photons (at least one of the strong field frequencies enters the susceptibility with the minus sign). Alternatively, enhancement for the highest-order harmonic generation (when all the photons are ''accumulated'') is minimal. The predicted phenomena bear information on spectral properties of both impurity molecules and a fractal. In particular, in the CARS spectra a narrow (with the natural width) resonant structure, which is proper to an isolated monomer of a fractal, is predicted to be observed. (orig.)
Optical nonlinearity enhancement with graphene-decorated silicon waveguides
Ishizawa, Atsushi; Kou, Rai; Goto, Takahiro; Tsuchizawa, Tai; Matsuda, Nobuyuki; Hitachi, Kenichi; Nishikawa, Tadashi; Yamada, Koji; Sogawa, Tetsuomi; Gotoh, Hideki
2017-04-01
Broadband on-chip optical frequency combs (OFCs) are important for expanding the functionality of photonic integrated circuits. Here, we demonstrate a huge local optical nonlinearity enhancement using graphene. A waveguide is decorated with graphene by precisely manipulating graphene’s area and position. Our approach simultaneously achieves both an extremely efficient supercontinuum and ultra-short pulse generation. With our graphene-decorated silicon waveguide (G-SWG), we have achieved enhanced spectral broadening of femtosecond pump pulses, along with an eightfold increase in the output optical intensity at a wavelength approximately 200 nm shorter than that of the pump pulses. We also found that this huge nonlinearity works as a compressor that effectively compresses pulse width from 80 to 15.7 fs. Our results clearly show the potential for our G-SWG to greatly boost the speed and capacity of future communications with lower power consumption, and our method will further decrease the required pump laser power because it can be applied to decorate various kinds of waveguides with various two-dimensional materials.
On Madelung systems in nonlinear optics: A reciprocal invariance
Rogers, Colin; Malomed, Boris
2018-05-01
The role of the de Broglie-Bohm potential, originally established as central to Bohmian quantum mechanics, is examined for two canonical Madelung systems in nonlinear optics. In a seminal case, a Madelung system derived by Wagner et al. via the paraxial approximation and in which the de Broglie-Bohm potential is present is shown to admit a multi-parameter class of what are here introduced as "q-gaussons." In the limit, as the Tsallis parameter q → 1, the q-gaussons are shown to lead to standard gausson solitons, as admitted by the logarithmic nonlinear Schrödinger equation encapsulating the Madelung system. The q-gaussons are obtained for optical media with dual power-law refractive index. In the second case, a Madelung system originally derived via an eikonal approximation in the context of laser beam propagation and in which the de Broglie Bohm term is neglected is shown to admit invariance under a novel class of two-parameter class of reciprocal transformations. Model optical laws analogous to the celebrated Kármán-Tsien law of classical gas dynamics are introduced.
Transmutation of skyrmions to half-solitons driven by the nonlinear optical spin Hall effect.
Flayac, H; Solnyshkov, D D; Shelykh, I A; Malpuech, G
2013-01-04
We show that the spin domains, generated in the linear optical spin Hall effect by the analog of spin-orbit interaction for exciton polaritons, are associated with the formation of a Skyrmion lattice. In the nonlinear regime, the spin anisotropy of the polariton-polariton interactions results in a spatial compression of the domains and in a transmutation of the Skyrmions into oblique half-solitons. This phase transition is associated with both the focusing of the spin currents and the emergence of a strongly anisotropic emission pattern.
Laboratory beam-plasma interactions: linear and nonlinear
International Nuclear Information System (INIS)
Christiansen, P.J.; Jain, V.K.; Bond, J.W.
1982-01-01
The present investigation is concerned with the configuration of a cool plasma (often magnetized axially) penetrated by an injected electron beam. The attempt is made to demonstrate that despite unavoidable scaling limitations, laboratory experiments can illuminate, in a controlled fashion, details of beam plasma interaction processes in a way which will never be possible in the space plasma physics. In view of the increasing interest in high frequency instabilities in the auroral zone, the possibilities for interesting cross fertilizations of the two fields appear to be extensive. The linear theory is considered along with low frequency couplings and indirect effects. Attention is given to the evidence for the existence of exponentially growing instabilities in beam plasma interactions. The consequences of such instabilities are also explored and some processes of nonlinear processes are discussed, taking into account quasi-linear effects, trapping effects, nonlinear effects, trapping effects, nonlinear wave-wave interactions, and self-modulation and cavitation. 80 references
Z-scan: A simple technique for determination of third-order optical nonlinearity
Energy Technology Data Exchange (ETDEWEB)
Singh, Vijender, E-mail: chahal-gju@rediffmail.com [Department of Applied Science, N.C. College of Engineering, Israna, Panipat-132107, Haryana (India); Aghamkar, Praveen, E-mail: p-aghamkar@yahoo.co.in [Department of Physics, Chaudhary Devi Lal University, Sirsa-125055, Haryana (India)
2015-08-28
Z-scan is a simple experimental technique to measure intensity dependent nonlinear susceptibilities of third-order nonlinear optical materials. This technique is used to measure the sign and magnitude of both real and imaginary part of the third order nonlinear susceptibility (χ{sup (3)}) of nonlinear optical materials. In this paper, we investigate third-order nonlinear optical properties of Ag-polymer composite film by using single beam z-scan technique with Q-switched, frequency doubled Nd: YAG laser (λ=532 nm) at 5 ns pulse. The values of nonlinear absorption coefficient (β), nonlinear refractive index (n{sub 2}) and third-order nonlinear optical susceptibility (χ{sup (3)}) of permethylazine were found to be 9.64 × 10{sup −7} cm/W, 8.55 × 10{sup −12} cm{sup 2}/W and 5.48 × 10{sup −10} esu, respectively.
Nonlinear polarization effects in a birefringent single mode optical fiber
International Nuclear Information System (INIS)
Ishiekwene, G.C.; Mensah, S.Y.; Brown, C.S.
2001-04-01
The nonlinear polarization effects in a birefringent single mode optical fiber is studied using Jacobi elliptic functions. We find that the polarization state of the propagating beam depends on the initial polarization as well as the intensity of the input light in a complicated way. The Stokes polarization parameters are either periodic or aperiodic depending on the value of the Jacobian modulus. Our calculations suggest that the effective beat length of the fiber can become infinite at a higher critical value of the input power when polarization dependent losses are considered. (author)
Dispersive shock waves in nonlinear and atomic optics
Directory of Open Access Journals (Sweden)
Kamchatnov Anatoly
2017-01-01
Full Text Available A brief review is given of dispersive shock waves observed in nonlinear optics and dynamics of Bose-Einstein condensates. The theory of dispersive shock waves is developed on the basis of Whitham modulation theory for various situations taking place in these two fields. In particular, the full classification is established for types of wave structures evolving from initial discontinuities for propagation of long light pulses in fibers with account of steepening effect and for dynamics of the polarization mode in two-component Bose-Einstein condensates.
Superradiance Effects in the Linear and Nonlinear Optical Response of Quantum Dot Molecules
Sitek, A.; Machnikowski, P.
2008-11-01
We calculate the linear optical response from a single quantum dot molecule and the nonlinear, four-wave-mixing response from an inhomogeneously broadened ensemble of such molecules. We show that both optical signals are affected by the coupling-dependent superradiance effect and by optical interference between the two polarizations. As a result, the linear and nonlinear responses are not identical.
Kuindersma, P.I.; Leijtens, X.J.M.; Zantvoort, van J.H.C.; Waardt, de H.
2012-01-01
We characterize integrated InP circuits for high speed ‘all-optical’ signal processing. Single chip circuits act as optical transistors. Transmodulation is performed by non-linear gain sections. Integrated tunable filters give signal equalization in time domain.
Non-linear electromagnetic interactions in thermal QED
International Nuclear Information System (INIS)
Brandt, F.T.; Frenkel, J.
1994-08-01
The behavior of the non-linear interactions between electromagnetic fields at high temperature is examined. It is shown that, in general, the log(T) dependence on the temperature of the Green functions is simply related to their UV behavior at zero-temperature. It is argued that the effective action describing the nonlinear thermal electromagnetic interactions has a finite limit as T -> ∞. This thermal action approaches, in the long wavelength limit, the negative of the corresponding zero-temperature action. (author). 12 refs, 1 fig
Nonlinear optical response of some Graphene oxide and Graphene fluoride derivatives
Liaros Nikolaos; Orfanos Ioannis; Papadakis Ioannis; Couris Stelios
2016-01-01
The nonlinear optical properties of two graphene derivatives, graphene oxide and graphene fluoride, are investigated by means of the Z-scan technique employing 35 ps and 4 ns, visible (532 nm) laser excitation. Both derivatives were found to exhibit significant third-order nonlinear optical response at both excitation regimes, with the nonlinear absorption being relatively stronger and concealing the presence of nonlinear refraction under ns excitation, while ps excita...
Dynamic nonlinear interaction of elastic plates on discrete supports
International Nuclear Information System (INIS)
Coutinho, A.L.G.A.; Landau, L.; Lima, E.C.P. de; Ebecken, N.F.F.
1984-01-01
A study on the dynamic nonlinear interaction of elastic plates using the finite element method is presented. The elastic plate is discretized by 4-node isoparametric Mindlin elements. The constitutive relation of the discrete supports can be any nonlinear curve given by pairs of force-displacement points. The nonlinear behaviour is represented by the overlay approach. This model also allows the simulation of a progressive decrease on the supports stiffnesses during load cycles. The dynamic nonlinear incremental movement equations are integrated by the Newmark implicit operator. Two alternatives for the incremental-iterative formulation are compared. The paper ends with a discussion of the advantages and limitations of the presented numerical models. (Author) [pt
A novel organic nonlinear optical crystal: Creatininium succinate
Energy Technology Data Exchange (ETDEWEB)
Thirumurugan, R.; Anitha, K., E-mail: singlecerystalxrd@gmail.ciom [School of Physics, Madurai Kamraj University, Madurai 625021 (India)
2015-06-24
A novel organic material complex of creatininium succinate (CS) has been synthesized and single crystals were grown by the reaction of creatinine and succinic acid from aqueous solution by employing the technique of slow evaporation at room temperature. The structure of the grown crystal has been elucidated using single crystal X-ray diffraction analysis and the structure was refined by least-squares method to R = 0.027 for 1840 reflections. FT-IR spectral investigation has been carried out to identify the various functional groups in the title compound. UV–Vis transmission was carried out which shows the crystal has a good optical transmittance in the visible region with lower cutoff wavelength around 220 nm. Nonlinear optical property of the crystal was confirmed by Kurtz-Perry powder technique.
1994-01-01
HOSOTTE: Alignement and Orientation of Chromophores by Optical Pumping 327 CELINE FIORINI, FABRICE CHARRA, JEAN-MICHEL NUNZI and PAUL RAIMOND...Normandin, R. L. Williams and M. Dion , Electron. Lett., 28, 1540 (1992). 6. D. Vakhshoori and S. Wang, Appl. Phys. Lett., 53, 347 (1988). 7. D. Vakhshoori, J
Molecular studies and plastic optical fiber device structures for nonlinear optical applications
Dirk, Carl W.; Nagarur, Aruna R.; Lu, Jin J.; Zhang, Lixia; Kalamegham, Priya; Fonseca, Joe; Gopalan, Saytha; Townsend, Scott; Gonzalez, Gabriel; Craig, Patrick; Rosales, Monica; Green, Leslie; Chan, Karen; Twieg, Robert J.; Ermer, Susan P.; Leung, Doris S.; Lovejoy, Steven M.; Lacroix, Suzanne; Godbout, Nicolas; Monette, Etienne
1995-10-01
Summarized are two project areas: First, the development of a quantitative structure property relationship for analyzing thermal decomposition differential scanning calorimetry data of electro-optic dyes is presented. The QSPR relationship suggest that thermal decomposition can be effectively correlated with structure by considering the kinds of atoms, their hybridization, and their nearest neighbor bonded atoms. Second, the simple preparation of clad plastic optical fibers (POF) is discussed with the intention of use for nonlinear optical applications. We discuss preparation techniques for single core and multiple core POF, and present some recent data on index profiles and the optimization of thermal stability in acrylate-based POF structures.
Emerging Low-Dimensional Materials for Nonlinear Optics and Ultrafast Photonics.
Liu, Xiaofeng; Guo, Qiangbing; Qiu, Jianrong
2017-04-01
Low-dimensional (LD) materials demonstrate intriguing optical properties, which lead to applications in diverse fields, such as photonics, biomedicine and energy. Due to modulation of electronic structure by the reduced structural dimensionality, LD versions of metal, semiconductor and topological insulators (TIs) at the same time bear distinct nonlinear optical (NLO) properties as compared with their bulk counterparts. Their interaction with short pulse laser excitation exhibits a strong nonlinear character manifested by NLO absorption, giving rise to optical limiting or saturated absorption associated with excited state absorption and Pauli blocking in different materials. In particular, the saturable absorption of these emerging LD materials including two-dimensional semiconductors as well as colloidal TI nanoparticles has recently been utilized for Q-switching and mode-locking ultra-short pulse generation across the visible, near infrared and middle infrared wavelength regions. Beside the large operation bandwidth, these ultrafast photonics applications are especially benefit from the high recovery rate as well as the facile processibility of these LD materials. The prominent NLO response of these LD materials have also provided new avenues for the development of novel NLO and photonics devices for all-optical control as well as optical circuits beyond ultrafast lasers. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Nonlinear optical oscillation dynamics in high-Q lithium niobate microresonators.
Sun, Xuan; Liang, Hanxiao; Luo, Rui; Jiang, Wei C; Zhang, Xi-Cheng; Lin, Qiang
2017-06-12
Recent advance of lithium niobate microphotonic devices enables the exploration of intriguing nonlinear optical effects. We show complex nonlinear oscillation dynamics in high-Q lithium niobate microresonators that results from unique competition between the thermo-optic nonlinearity and the photorefractive effect, distinctive to other device systems and mechanisms ever reported. The observed phenomena are well described by our theory. This exploration helps understand the nonlinear optical behavior of high-Q lithium niobate microphotonic devices which would be crucial for future application of on-chip nonlinear lithium niobate photonics.
Characterizing the Statistics of a Bunch of Optical Pulses Using a Nonlinear Optical Loop Mirror
Directory of Open Access Journals (Sweden)
Olivier Pottiez
2015-01-01
Full Text Available We propose in this work a technique for determining the amplitude distribution of a wave packet containing a large number of short optical pulses with different amplitudes. The technique takes advantage of the fast response of the optical Kerr effect in a fiber nonlinear optical loop mirror (NOLM. Under some assumptions, the statistics of the pulses can be determined from the energy transfer characteristic of the packet through the NOLM, which can be measured with a low-frequency detection setup. The statistical distribution is retrieved numerically by approximating the solution of a system of nonlinear algebraic equations using the least squares method. The technique is demonstrated numerically in the case of a packet of solitons.
Nonlinear optical spectroscopy of isotropic and anisotropic metallic nanocomposites
Energy Technology Data Exchange (ETDEWEB)
Fernandez-Hernandez, R C; Gleason-Villagran, R; Cheang-Wong, J C; Crespo-Sosa, A; Rodriguez-Fernandez, L; Lopez-Suarez, A; Oliver, A; Reyes-Esqueda, J A [Instituto de Fisica, Universidad Nacional Autonoma de Mexico, Mexico, D. F. 04510 (Mexico); Torres-Torres, C [Seccion de Estudios de Posgrado e Investigacion, ESIME-Zacatenco, Instituto Politecnico Nacional, Mexico, D. F. 07338 (Mexico); Rangel-Rojo, R, E-mail: reyes@fisica.unam.mx [CICESE/Depto. de Optica, A.P. 360, Ensenada, B. C. 22860 (Mexico)
2011-01-01
In this work, we studied the nonlinear absorption and refraction of isotropic and anisotropic metallic nanocomposites, which consist of Au and Ag nanoparticles (NPs) embedded in matrices of SiO{sub 2}. We performed this study at different wavelengths using the Z-scan technique in the picosecond regime. The wavelengths were selected accordingly to the absorption spectra of the nanocomposites, choosing wavelengths into the inter- and intra-band transitions regions, including the surface plasmon (SP) resonance, as well as in the transparent region. For the anisotropic nanocomposites, the polarization and the incident angle were varied in order to evaluate the different components of the third order susceptibility tensor, {chi}{sup (3)}. We observed dramatic changes of sign for both, nonlinear refraction and absorption, when passing from Au to Ag and/or varying the wave length. The results accentuate the importance of the hot-electrons contribution to the nonlinear optical response at this temporal regime, when compared to inter-band and intra-band transitions contributions.
Nonlinear optical spectroscopy of isotropic and anisotropic metallic nanocomposites
International Nuclear Information System (INIS)
Fernandez-Hernandez, R C; Gleason-Villagran, R; Cheang-Wong, J C; Crespo-Sosa, A; Rodriguez-Fernandez, L; Lopez-Suarez, A; Oliver, A; Reyes-Esqueda, J A; Torres-Torres, C; Rangel-Rojo, R
2011-01-01
In this work, we studied the nonlinear absorption and refraction of isotropic and anisotropic metallic nanocomposites, which consist of Au and Ag nanoparticles (NPs) embedded in matrices of SiO 2 . We performed this study at different wavelengths using the Z-scan technique in the picosecond regime. The wavelengths were selected accordingly to the absorption spectra of the nanocomposites, choosing wavelengths into the inter- and intra-band transitions regions, including the surface plasmon (SP) resonance, as well as in the transparent region. For the anisotropic nanocomposites, the polarization and the incident angle were varied in order to evaluate the different components of the third order susceptibility tensor, χ (3) . We observed dramatic changes of sign for both, nonlinear refraction and absorption, when passing from Au to Ag and/or varying the wave length. The results accentuate the importance of the hot-electrons contribution to the nonlinear optical response at this temporal regime, when compared to inter-band and intra-band transitions contributions.
Fabrication of Metallic Quantum Dot Arrays For Nanoscale Nonlinear Optics
McMahon, M. D.; Hmelo, A. B.; Lopez Magruder, R., III; Weller Haglund, R. A., Jr.; Feldman, L. C.
2003-03-01
Ordered arrays of metal nanocrystals embedded in or sequestered on dielectric hosts have potential applications as elements of nonlinear or near-field optical circuits, as sensitizers for fluorescence emitters and photo detectors, and as anchor points for arrays of biological molecules. Metal nanocrystals are strongly confined electronic systems with size-, shape and spatial orientation-dependent optical responses. At the smallest scales (below about 15 nm diameter), their band structure is drastically altered by the small size of the system, and the reduced population of conduction-band electrons. Here we report on the fabrication of two-dimensional ordered metallic nanocrystal arrays, and one-dimensional nanocrystal-loaded waveguides for optical investigations. We have employed strategies for synthesizing metal nanocrystal composites that capitalize on the best features of focused ion beam (FIB) machining and pulsed laser deposition (PLD). The FIB generates arrays of specialized sites; PLD vapor deposition results in the directed self-assembly of Ag nanoparticles nucleated at the FIB generated sites on silicon substrates. We present results based on the SEM, AFM and optical characterization of prototype composites. This research has been supported by the U.S. Department of Energy under grant DE-FG02-01ER45916.
Computational Modeling of Ultrafast Pulse Propagation in Nonlinear Optical Materials
Goorjian, Peter M.; Agrawal, Govind P.; Kwak, Dochan (Technical Monitor)
1996-01-01
There is an emerging technology of photonic (or optoelectronic) integrated circuits (PICs or OEICs). In PICs, optical and electronic components are grown together on the same chip. rib build such devices and subsystems, one needs to model the entire chip. Accurate computer modeling of electromagnetic wave propagation in semiconductors is necessary for the successful development of PICs. More specifically, these computer codes would enable the modeling of such devices, including their subsystems, such as semiconductor lasers and semiconductor amplifiers in which there is femtosecond pulse propagation. Here, the computer simulations are made by solving the full vector, nonlinear, Maxwell's equations, coupled with the semiconductor Bloch equations, without any approximations. The carrier is retained in the description of the optical pulse, (i.e. the envelope approximation is not made in the Maxwell's equations), and the rotating wave approximation is not made in the Bloch equations. These coupled equations are solved to simulate the propagation of femtosecond optical pulses in semiconductor materials. The simulations describe the dynamics of the optical pulses, as well as the interband and intraband.
Mechanism of large optical nonlinearity in gold nanoparticle films.
Mirza, I; McCloskey, D; Blau, W J; Lunney, J G
2018-04-01
The Z-scan technique, using femtosecond (fs) laser pulses at 1480 nm laser pulses, was used to measure the nonlinear optical properties of gold (Au) nanoparticle (NP) films made by both nanosecond (ns) and fs pulsed laser deposition (PLD) in vacuum. At irradiance levels of 1×10 12 Wm -2 , the ns-PLD films displayed induced absorption with β=4×10 -5 mW -1 , and a negative lensing effect with n 2 =-4.7×10 -11 m 2 W -1 with somewhat smaller values for the fs-PLD films. These values of n 2 imply an unphysically large change in the real part of the refractive index, demonstrating the need to take account of nonlinear changes of the Fresnel coefficients and multiple beam interference in Z-scan measurements on nanoscale films. Following this approach, the Z-scan observations were analyzed to determine the effective complex refractive index of the NP film at high irradiance. It appears that at high irradiance the NP film behaves as a metal, while at low irradiance it behaves as a low-loss dielectric. Thus, it is conjectured that, for high irradiance near the waist of the Z-scan laser beam, laser driven electron tunneling between NPs gives rise to metal-like optical behavior.
How nonlinear optics can merge interferometry for high resolution imaging
Ceus, D.; Reynaud, F.; Tonello, A.; Delage, L.; Grossard, L.
2017-11-01
High resolution stellar interferometers are very powerful efficient instruments to get a better knowledge of our Universe through the spatial coherence analysis of the light. For this purpose, the optical fields collected by each telescope Ti are mixed together. From the interferometric pattern, two expected information called the contrast Cij and the phase information φij are extracted. These information lead to the Vij, called the complex visibility, with Vij=Cijexp(jφij). For each telescope doublet TiTj, it is possible to get a complex visibility Vij. The Zernike Van Cittert theorem gives a relationship between the intensity distribution of the object observed and the complex visibility. The combination of the acquired complex visibilities and a reconstruction algorithm allows imaging reconstruction. To avoid lots of technical difficulties related to infrared optics (components transmission, thermal noises, thermal cooling…), our team proposes to explore the possibility of using nonlinear optical techniques. This is a promising alternative detection technique for detecting infrared optical signals. This way, we experimentally demonstrate that frequency conversion does not result in additional bias on the interferometric data supplied by a stellar interferometer. In this presentation, we report on wavelength conversion of the light collected by each telescope from the infrared domain to the visible. The interferometric pattern is observed in the visible domain with our, so called, upconversion interferometer. Thereby, one can benefit from mature optical components mainly used in optical telecommunications (waveguide, coupler, multiplexer…) and efficient low-noise detection schemes up to the single-photon counting level.
Directory of Open Access Journals (Sweden)
Virginijus Barzda
2013-09-01
Full Text Available Differential polarization nonlinear optical microscopy has the potential to become an indispensable tool for structural investigations of ordered biological assemblies and microcrystalline aggregates. Their microscopic organization can be probed through fast and sensitive measurements of nonlinear optical signal anisotropy, which can be achieved with microscopic spatial resolution by using time-multiplexed pulsed laser beams with perpendicular polarization orientations and photon-counting detection electronics for signal demultiplexing. In addition, deformable membrane mirrors can be used to correct for optical aberrations in the microscope and simultaneously optimize beam overlap using a genetic algorithm. The beam overlap can be achieved with better accuracy than diffraction limited point-spread function, which allows to perform polarization-resolved measurements on the pixel-by-pixel basis. We describe a newly developed differential polarization microscope and present applications of the differential microscopy technique for structural studies of collagen and cellulose. Both, second harmonic generation, and fluorescence-detected nonlinear absorption anisotropy are used in these investigations. It is shown that the orientation and structural properties of the fibers in biological tissue can be deduced and that the orientation of fluorescent molecules (Congo Red, which label the fibers, can be determined. Differential polarization microscopy sidesteps common issues such as photobleaching and sample movement. Due to tens of megahertz alternating polarization of excitation pulses fast data acquisition can be conveniently applied to measure changes in the nonlinear signal anisotropy in dynamically changing in vivo structures.
Nonlinear interaction of the surface waves at a plasma boundary
International Nuclear Information System (INIS)
Dolgopolov, V.V.; El-Naggar, I.A.; Hussein, A.M.; Khalil, Sh.M.
1976-01-01
Amplitudes of electromagnetic waves with combination frequencies, radiating from the plasma boundary due to nonlinear interaction of the surface waves, have been found. Previous papers on this subject did not take into account that the tangential components of the electric field of waves with combination frequencies were discontinuous at the plasma boundary. (Auth.)
Non-Linear Interactive Stories in Computer Games
DEFF Research Database (Denmark)
Bangsø, Olav; Jensen, Ole Guttorm; Kocka, Tomas
2003-01-01
The paper introduces non-linear interactive stories (NOLIST) as a means to generate varied and interesting stories for computer games automatically. We give a compact representation of a NOLIST based on the specification of atomic stories, and show how to build an object-oriented Bayesian network...
The nonlinear Schrödinger equation singular solutions and optical collapse
Fibich, Gadi
2015-01-01
This book is an interdisciplinary introduction to optical collapse of laser beams, which is modelled by singular (blow-up) solutions of the nonlinear Schrödinger equation. With great care and detail, it develops the subject including the mathematical and physical background and the history of the subject. It combines rigorous analysis, asymptotic analysis, informal arguments, numerical simulations, physical modelling, and physical experiments. It repeatedly emphasizes the relations between these approaches, and the intuition behind the results. The Nonlinear Schrödinger Equation will be useful to graduate students and researchers in applied mathematics who are interested in singular solutions of partial differential equations, nonlinear optics and nonlinear waves, and to graduate students and researchers in physics and engineering who are interested in nonlinear optics and Bose-Einstein condensates. It can be used for courses on partial differential equations, nonlinear waves, and nonlinear optics. Gadi Fib...
Directory of Open Access Journals (Sweden)
Arnaud Mussot
2014-03-01
Full Text Available The discovery of the Fermi-Pasta-Ulam (FPU recurrence phenomenon in the 1950 s was a major step in science that later led to the discovery of solitons in nonlinear physics. More recently, it was shown that optical fibers can serve as a medium for observing the FPU phenomenon. In the present work, we have found experimentally and numerically that in the low-dispersion region of an optical fiber, the recurrence is strongly influenced by the third-order-dispersion (TOD term. Namely, the presence of TOD leads to several disappearances and recoveries of the FPU recurrence when the central frequency of the pump wave is varied. The effect is highly nontrivial and can be explained in terms of reversible and irreversible losses caused by Cherenkov radiations interacting with a multiplicity of modes sharing the optical energy in the process of its partition.
Nonlinear effects in optical pumping of a cold and slow atomic beam
Porfido, N.
2015-10-12
By photoionizing hyperfine (HF) levels of the Cs state 62P3/2 in a slow and cold atom beam, we find how their population depends on the excitation laser power. The long time (around 180μs) spent by the slow atoms inside the resonant laser beam is large enough to enable exploration of a unique atom-light interaction regime heavily affected by time-dependent optical pumping. We demonstrate that, under such conditions, the onset of nonlinear effects in the population dynamics and optical pumping occurs at excitation laser intensities much smaller than the conventional respective saturation values. The evolution of population within the HF structure is calculated by numerical integration of the multilevel optical Bloch equations. The agreement between numerical results and experiment outcomes is excellent. All main features in the experimental findings are explained by the occurrence of “dark” and “bright” resonances leading to power-dependent branching coefficients.
NON-LINEAR MODELING OF THE RHIC INTERACTION REGIONS
International Nuclear Information System (INIS)
TOMAS, R.; FISCHER, W.; JAIN, A.; LUO, Y.; PILAT, F.
2004-01-01
For RHIC's collision lattices the dominant sources of transverse non-linearities are located in the interaction regions. The field quality is available for most of the magnets in the interaction regions from the magnetic measurements, or from extrapolations of these measurements. We discuss the implementation of these measurements in the MADX models of the Blue and the Yellow rings and their impact on beam stability
Third order nonlinear optical properties of a paratellurite single crystal
Duclère, J.-R.; Hayakawa, T.; Roginskii, E. M.; Smirnov, M. B.; Mirgorodsky, A.; Couderc, V.; Masson, O.; Colas, M.; Noguera, O.; Rodriguez, V.; Thomas, P.
2018-05-01
The (a,b) plane angular dependence of the third-order nonlinear optical susceptibility, χ(3) , of a c-cut paratellurite (α-TeO2) single crystal was quantitatively evaluated here by the Z-scan technique, using a Ti:sapphire femtosecond laser operated at 800 nm. In particular, the mean value Re( ⟨χ(3)⟩a,b )(α-TeO2) of the optical tensor has been extracted from such experiments via a direct comparison with the data collected for a fused silica reference glass plate. A R e (⟨χ(3)⟩(a,b )(α-TeO2)):R e (χ(3))(SiO2 glass) ratio roughly equal to 49.1 is found, and our result compares thus very favourably with the unique experimental value (a ratio of ˜50) reported by Kim et al. [J. Am. Ceram. Soc. 76, 2486 (1993)] for a pure TeO2 glass. In addition, it is shown that the angular dependence of the phase modulation within the (a,b) plane can be fully understood in the light of the strong dextro-rotatory power known for TeO2 materials. Taking into account the optical activity, some analytical model serving to estimate the diagonal and non-diagonal components of the third order nonlinear susceptibility tensor has been thus developed. Finally, Re( χxxxx(3) ) and Re( χxxyy(3) ) values of 95.1 ×10-22 m 2/V2 and 42.0 ×10-22 m2/V2 , respectively, are then deduced for a paratellurite single crystal, considering fused silica as a reference.
Design and optimization of carbon-nanotube-material/dielectric hybrid nonlinear optical waveguides
International Nuclear Information System (INIS)
Zhao, Xin; Zheng, Zheng; Lu, Zhiting; Zhu, Jinsong; Zhou, Tao
2011-01-01
The nonlinear optical characteristics of highly nonlinear waveguides utilizing carbon nanotube composite materials are investigated theoretically. The extremely high nonlinearity and relatively high loss of the carbon nanotube materials are shown to greatly affect the performance of such waveguides for nonlinear optical applications, in contrast to waveguides using conventional nonlinear materials. Different configurations based on applying the carbon nanotube materials to the popular ridge and buried waveguides are thoroughly studied, and the optimal geometries are derived through simulations. It is shown that, though the nonlinear coefficient is often huge for these waveguides, the loss characteristics can significantly limit the maximum achievable accumulated nonlinearity, e.g. the maximum nonlinear phase shift. Our results suggest that SOI-based high-index-contrast, carbon nanotube cladding waveguides, rather than the currently demonstrated low-contrast waveguides, could hold the promise of achieving significantly higher accumulated nonlinearity
International Nuclear Information System (INIS)
Carrillo-Delgado, C; Torres-Torres, C; García-Merino, J A; García-Gil, C I; Khomenko, A V; Trejo-Valdez, M; Martínez-Gutiérrez, H; Torres-Martínez, R
2016-01-01
Measurements of the third-order nonlinear optical properties exhibited by a ZnO thin solid film deposited on a SnO 2 substrate are presented. The samples were prepared by a spray pyrolysis processing route. Scanning electron microscopy analysis and UV–Vis spectroscopy studies were carried out. The picosecond response at 1064 nm was explored by the z-scan technique. A large optical Kerr effect with two-photon absorption was obtained. The inhibition of the nonlinear optical absorption together with a noticeable enhancement in the optical Kerr effect in the sample was achieved by the incorporation of Au nanoparticles into the ZnO film. Additionally, a two-wave mixing configuration at 532 nm was performed and an optical Kerr effect was identified as the main cause of the nanosecond third-order optical nonlinearity. The relaxation time of the photothermal response of the sample was estimated to be about 1 s when the sample was excited by nanosecond single-shots. The rotation of the sample during the nanosecond two-wave mixing experiments was analyzed. It was stated that a non-monotonic relation between rotating frequency and pulse repetition rate governs the thermal contribution to the nonlinear refractive index exhibited by a rotating film. Potential applications for switching photothermal interactions in rotating samples can be contemplated. A rotary logic system dependent on Kerr transmittance in a two-wave mixing experiment was proposed. (paper)
Linear and nonlinear interactions in the dark sector
International Nuclear Information System (INIS)
Chimento, Luis P.
2010-01-01
We investigate models of interacting dark matter and dark energy for the Universe in a spatially flat Friedmann-Robertson-Walker space-time. We find the 'source equation' for the total energy density and determine the energy density of each dark component. We introduce an effective one-fluid description to evidence that interacting and unified models are related to each other, analyze the effective model, and obtain the attractor solutions. We study linear and nonlinear interactions, the former comprises a linear combination of the dark matter and dark energy densities, their first derivatives, the total energy density, its first and second derivatives, and a function of the scale factor. The latter is a possible generalization of the linear interaction consisting of an aggregate of the above linear combination and a significant nonlinear term built with a rational function of the dark matter and dark energy densities homogeneous of degree 1. We solve the evolution equations of the dark components for both interactions and examine exhaustively several examples. There exist cases where the effective one-fluid description produces different alternatives to the ΛCDM model and cases where the problem of coincidence is alleviated. In addition, we find that some nonlinear interactions yield an effective one-fluid model with a Chaplygin gas equation of state, whereas others generate cosmological models with de Sitter and power-law expansions. We show that a generic nonlinear interaction induces an effective equation of state which depends on the scale factor in the same way as the variable modified Chaplygin gas model, giving rise to the 'relaxed Chaplygin gas model'.
Permanent dipole moments and damping in nonlinear optics. A quantum electrodynamic description
International Nuclear Information System (INIS)
Davila-Smith, L.C.
1999-01-01
Based on the well-known transformation of the electric-dipole interaction, different nonlinear optical processes are analysed. The transformation provides a convenient means for ascertaining the effects of permanent dipoles on the optical behaviour of systems with a response dominated by two energy levels. By establishing the general validity of the procedure for parametric and non-parametric processes, it is shown how the detailed structure of the optical nonlinearity can be ascertained, based on a novel interpretation of the relevant quantum electrodynamical Feynman diagrams. This transformation is used to analysed a novel five-wave mixing process, which is also developed in this thesis. This process is of considerable interest for its involvement in the generation of even harmonics in isotropic media. Also, the flexibility in the beam geometry affords considerable scope for the study of the polarisation and angular dependence. Finally, a general study of the effects of resonance in matter-radiation interactions is given, justifying the phenomenological incorporation of the damping addenda. The two alternative convention used when the damping is introduced are discussed, showing that both conventions lead to different physical results. Based on these studies the resonance effects are considered in relation to different multiphoton processes. (author)
FDTD modeling of anisotropic nonlinear optical phenomena in silicon waveguides.
Dissanayake, Chethiya M; Premaratne, Malin; Rukhlenko, Ivan D; Agrawal, Govind P
2010-09-27
A deep insight into the inherent anisotropic optical properties of silicon is required to improve the performance of silicon-waveguide-based photonic devices. It may also lead to novel device concepts and substantially extend the capabilities of silicon photonics in the future. In this paper, for the first time to the best of our knowledge, we present a three-dimensional finite-difference time-domain (FDTD) method for modeling optical phenomena in silicon waveguides, which takes into account fully the anisotropy of the third-order electronic and Raman susceptibilities. We show that, under certain realistic conditions that prevent generation of the longitudinal optical field inside the waveguide, this model is considerably simplified and can be represented by a computationally efficient algorithm, suitable for numerical analysis of complex polarization effects. To demonstrate the versatility of our model, we study polarization dependence for several nonlinear effects, including self-phase modulation, cross-phase modulation, and stimulated Raman scattering. Our FDTD model provides a basis for a full-blown numerical simulator that is restricted neither by the single-mode assumption nor by the slowly varying envelope approximation.
Optical Asymmetry and Nonlinear Light Scattering from Colloidal Gold Nanorods.
Lien, Miao-Bin; Kim, Ji-Young; Han, Myung-Geun; Chang, You-Chia; Chang, Yu-Chung; Ferguson, Heather J; Zhu, Yimei; Herzing, Andrew A; Schotland, John C; Kotov, Nicholas A; Norris, Theodore B
2017-06-27
A systematic study is presented of the intensity-dependent nonlinear light scattering spectra of gold nanorods under resonant excitation of the longitudinal surface plasmon resonance (SPR). The spectra exhibit features due to coherent second and third harmonic generation as well as a broadband feature that has been previously attributed to multiphoton photoluminescence arising primarily from interband optical transitions in the gold. A detailed study of the spectral dependence of the scaling of the scattered light with excitation intensity shows unexpected scaling behavior of the coherent signals, which is quantitatively accounted for by optically induced damping of the SPR mode through a Fermi liquid model of the electronic scattering. The broadband feature is shown to arise not from luminescence, but from scattering of the second-order longitudinal SPR mode with the electron gas, where efficient excitation of the second order mode arises from an optical asymmetry of the nanorod. The electronic-temperature-dependent plasmon damping and the Fermi-Dirac distribution together determine the intensity dependence of the broadband emission, and the structure-dependent absorption spectrum determines the spectral shape through the fluctuation-dissipation theorem. Hence a complete self-consistent picture of both coherent and incoherent light scattering is obtained with a single set of physical parameters.
Complete elimination of nonlinear light-matter interactions with broadband ultrafast laser pulses
DEFF Research Database (Denmark)
Shu, Chuan-Cun; Dong, Daoyi; Petersen, Ian R.
2017-01-01
optical effects, however, the probability of pure single-photon absorption is usually very low, which is particularly pertinent in the case of strong ultrafast laser pulses with broad bandwidth. Here we demonstrate theoretically a counterintuitive coherent single-photon absorption scheme by eliminating...... nonlinear interactions of ultrafast laser pulses with quantum systems. That is, a completely linear response of the system with respect to the spectral energy density of the incident light at the transition frequency can be obtained for all transition probabilities between 0 and 100% in multilevel quantum...... systems. To that end, a multiobjective optimization algorithm is developed to find an optimal spectral phase of an ultrafast laser pulse, which is capable of eliminating all possible nonlinear optical responses while maximizing the probability of single-photon absorption between quantum states. This work...
Dynamical soil-structure interactions: influence of soil behaviour nonlinearities
International Nuclear Information System (INIS)
Gandomzadeh, Ali
2011-01-01
The interaction of the soil with the structure has been largely explored the assumption of material and geometrical linearity of the soil. Nevertheless, for moderate or strong seismic events, the maximum shear strain can easily reach the elastic limit of the soil behavior. Considering soil-structure interaction, the nonlinear effects may change the soil stiffness at the base of the structure and therefore energy dissipation into the soil. Consequently, ignoring the nonlinear characteristics of the dynamic soil-structure interaction (DSSI) this phenomenon could lead to erroneous predictions of structural response. The goal of this work is to implement a fully nonlinear constitutive model for soils into a numerical code in order to investigate the effect of soil nonlinearity on dynamic soil structure interaction. Moreover, different issues are taken into account such as the effect of confining stress on the shear modulus of the soil, initial static condition, contact elements in the soil-structure interface, etc. During this work, a simple absorbing layer method based on a Rayleigh/Caughey damping formulation, which is often already available in existing Finite Element softwares, is also presented. The stability conditions of the wave propagation problems are studied and it is shown that the linear and nonlinear behavior are very different when dealing with numerical dispersion. It is shown that the 10 points per wavelength rule, recommended in the literature for the elastic media is not sufficient for the nonlinear case. The implemented model is first numerically verified by comparing the results with other known numerical codes. Afterward, a parametric study is carried out for different types of structures and various soil profiles to characterize nonlinear effects. Different features of the DSSI are compared to the linear case: modification of the amplitude and frequency content of the waves propagated into the soil, fundamental frequency, energy dissipation in
LINEAR AND NONLINEAR CORRECTIONS IN THE RHIC INTERACTION REGIONS
International Nuclear Information System (INIS)
PILAT, F.; CAMERON, P.; PTITSYN, V.; KOUTCHOUK, J.P.
2002-01-01
A method has been developed to measure operationally the linear and non-linear effects of the interaction region triplets, that gives access to the multipole content through the action kick, by applying closed orbit bumps and analyzing tune and orbit shifts. This technique has been extensively tested and used during the RHIC operations in 2001. Measurements were taken at 3 different interaction regions and for different focusing at the interaction point. Non-linear effects up to the dodecapole have been measured as well as the effects of linear, sextupolar and octupolar corrections. An analysis package for the data processing has been developed that through a precise fit of the experimental tune shift data (measured by a phase lock loop technique to better than 10 -5 resolution) determines the multipole content of an IR triplet
Zeng, Shihao; Chen, Manna; Zhang, Ting; Hu, Wei; Guo, Qi; Lu, Daquan
2018-01-01
We illuminate an analytical model of soliton interactions in lead glass by analogizing to a gravitational force system. The orbits of spiraling solitons under a long-range interaction are given explicitly and demonstrated to follow Newton's second law of motion and the Binet equation by numerical simulations. The condition for circular orbits is obtained and the oscillating orbits are proved not to be closed. We prove the analogy between the nonlocal nonlinear optical system and gravitational system and specify the quantitative relation of the quantity between the two models.
Marudhu, G.; Krishnan, S.; Palanichamy, M.
2016-03-01
A novel nonlinear optical crystal of 4-Aminopyridinium monophthalate (4-APMP) was grown by slow evaporation technique using methanol as solvent. Single crystal X-ray diffraction analysis confirms that the grown crystal belongs to orthorhombic system. The presence of functional groups was qualitatively determined by FTIR analysis. The optical absorption studies reveal very low absorption in the entire visible region. The fluorescence emission spectrum shows the emission is in blue region. The thermal stability of the grown crystal is found to be around 197.2 °C. The SHG efficiency of the grown crystal is found to be 1.1 times than that of KDP crystals.
The Particle Beam Optics Interactive Computer Laboratory
International Nuclear Information System (INIS)
Gillespie, G.H.; Hill, B.W.; Brown, N.A.; Babcock, R.C.; Martono, H.; Carey, D.C.
1997-01-01
The Particle Beam Optics Interactive Computer Laboratory (PBO Lab) is an educational software concept to aid students and professionals in learning about charged particle beams and particle beam optical systems. The PBO Lab is being developed as a cross-platform application and includes four key elements. The first is a graphic user interface shell that provides for a highly interactive learning session. The second is a knowledge database containing information on electric and magnetic optics transport elements. The knowledge database provides interactive tutorials on the fundamental physics of charged particle optics and on the technology used in particle optics hardware. The third element is a graphical construction kit that provides tools for students to interactively and visually construct optical beamlines. The final element is a set of charged particle optics computational engines that compute trajectories, transport beam envelopes, fit parameters to optical constraints and carry out similar calculations for the student designed beamlines. The primary computational engine is provided by the third-order TRANSPORT code. Augmenting TRANSPORT is the multiple ray tracing program TURTLE and a first-order matrix program that includes a space charge model and support for calculating single particle trajectories in the presence of the beam space charge. This paper describes progress on the development of the PBO Lab. copyright 1997 American Institute of Physics
The Particle Beam Optics Interactive Computer Laboratory
International Nuclear Information System (INIS)
Gillespie, George H.; Hill, Barrey W.; Brown, Nathan A.; Babcock, R. Chris; Martono, Hendy; Carey, David C.
1997-01-01
The Particle Beam Optics Interactive Computer Laboratory (PBO Lab) is an educational software concept to aid students and professionals in learning about charged particle beams and particle beam optical systems. The PBO Lab is being developed as a cross-platform application and includes four key elements. The first is a graphic user interface shell that provides for a highly interactive learning session. The second is a knowledge database containing information on electric and magnetic optics transport elements. The knowledge database provides interactive tutorials on the fundamental physics of charged particle optics and on the technology used in particle optics hardware. The third element is a graphical construction kit that provides tools for students to interactively and visually construct optical beamlines. The final element is a set of charged particle optics computational engines that compute trajectories, transport beam envelopes, fit parameters to optical constraints and carry out similar calculations for the student designed beamlines. The primary computational engine is provided by the third-order TRANSPORT code. Augmenting TRANSPORT is the multiple ray tracing program TURTLE and a first-order matrix program that includes a space charge model and support for calculating single particle trajectories in the presence of the beam space charge. This paper describes progress on the development of the PBO Lab
An integrated nonlinear optical loop mirror in silicon photonics for all-optical signal processing
Directory of Open Access Journals (Sweden)
Zifei Wang
2018-02-01
Full Text Available The nonlinear optical loop mirror (NOLM has been studied for several decades and has attracted considerable attention for applications in high data rate optical communications and all-optical signal processing. The majority of NOLM research has focused on silica fiber-based implementations. While various fiber designs have been considered to increase the nonlinearity and manage dispersion, several meters to hundreds of meters of fiber are still required. On the other hand, there is increasing interest in developing photonic integrated circuits for realizing signal processing functions. In this paper, we realize the first-ever passive integrated NOLM in silicon photonics and demonstrate its application for all-optical signal processing. In particular, we show wavelength conversion of 10 Gb/s return-to-zero on-off keying (RZ-OOK signals over a wavelength range of 30 nm with error-free operation and a power penalty of less than 2.5 dB, we achieve error-free nonreturn to zero (NRZ-to-RZ modulation format conversion at 10 Gb/s also with a power penalty of less than 2.8 dB, and we obtain error-free all-optical time-division demultiplexing of a 40 Gb/s RZ-OOK data signal into its 10 Gb/s tributary channels with a maximum power penalty of 3.5 dB.
Superior optical nonlinearity of an exceptional fluorescent stilbene dye
Energy Technology Data Exchange (ETDEWEB)
He, Tingchao [College of Physics Science and Technology, Shenzhen University, Shenzhen 518060 (China); Division of Physics and Applied Physics, Centre for Disruptive Photonic Technologies (CDPT), School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore 637371 (Singapore); Sreejith, Sivaramapanicker; Zhao, Yanli [Division of Chemistry and Biological Chemistry, School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore 637371 (Singapore); Gao, Yang; Grimsdale, Andrew C. [School of Materials Science and Engineering, Nanyang Technological University, Singapore, Singapore 639798 (Singapore); Lin, Xiaodong, E-mail: linxd@szu.edu.cn, E-mail: hdsun@ntu.edu.sg [College of Physics Science and Technology, Shenzhen University, Shenzhen 518060 (China); Sun, Handong, E-mail: linxd@szu.edu.cn, E-mail: hdsun@ntu.edu.sg [Division of Physics and Applied Physics, Centre for Disruptive Photonic Technologies (CDPT), School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore 637371 (Singapore)
2015-03-16
Strong multiphoton absorption and harmonic generation in organic fluorescent chromophores are, respectively, significant in many fields of research. However, most of fluorescent chromophores fall short of the full potential due to the absence of the combination of such different nonlinear upconversion behaviors. Here, we demonstrate that an exceptional fluorescent stilbene dye could exhibit efficient two- and three-photon absorption under the excitation of femtosecond pulses in solution phase. Benefiting from its biocompatibility and strong excited state absorption behavior, in vitro two-photon bioimaging and superior optical limiting have been exploited, respectively. Simultaneously, the chromophore could generate efficient three-photon excited fluorescence and third-harmonic generation (THG) when dispersed into PMMA film, circumventing the limitations of classical fluorescent chromophores. Such chromophore may find application in the production of coherent light sources of higher photon energy. Moreover, the combination of three-photon excited fluorescence and THG can be used in tandem to provide complementary information in biomedical studies.
Femtojoule-scale all-optical latching and modulation via cavity nonlinear optics.
Kwon, Yeong-Dae; Armen, Michael A; Mabuchi, Hideo
2013-11-15
We experimentally characterize Hopf bifurcation phenomena at femtojoule energy scales in a multiatom cavity quantum electrodynamical (cavity QED) system and demonstrate how such behaviors can be exploited in the design of all-optical memory and modulation devices. The data are analyzed by using a semiclassical model that explicitly treats heterogeneous coupling of atoms to the cavity mode. Our results highlight the interest of cavity QED systems for ultralow power photonic signal processing as well as for fundamental studies of mesoscopic nonlinear dynamics.
Navarrete-Benlloch, Carlos; Roldán, Eugenio; Chang, Yue; Shi, Tao
2014-10-06
Nonlinear optical cavities are crucial both in classical and quantum optics; in particular, nowadays optical parametric oscillators are one of the most versatile and tunable sources of coherent light, as well as the sources of the highest quality quantum-correlated light in the continuous variable regime. Being nonlinear systems, they can be driven through critical points in which a solution ceases to exist in favour of a new one, and it is close to these points where quantum correlations are the strongest. The simplest description of such systems consists in writing the quantum fields as the classical part plus some quantum fluctuations, linearizing then the dynamical equations with respect to the latter; however, such an approach breaks down close to critical points, where it provides unphysical predictions such as infinite photon numbers. On the other hand, techniques going beyond the simple linear description become too complicated especially regarding the evaluation of two-time correlators, which are of major importance to compute observables outside the cavity. In this article we provide a regularized linear description of nonlinear cavities, that is, a linearization procedure yielding physical results, taking the degenerate optical parametric oscillator as the guiding example. The method, which we call self-consistent linearization, is shown to be equivalent to a general Gaussian ansatz for the state of the system, and we compare its predictions with those obtained with available exact (or quasi-exact) methods. Apart from its operational value, we believe that our work is valuable also from a fundamental point of view, especially in connection to the question of how far linearized or Gaussian theories can be pushed to describe nonlinear dissipative systems which have access to non-Gaussian states.
Third-order nonlinear optical properties of ADP crystal
Wang, Mengxia; Wang, Zhengping; Chai, Xiangxu; Sun, Yuxiang; Sui, Tingting; Sun, Xun; Xu, Xinguang
2018-05-01
By using the Z-scan method, we investigated the third-order nonlinear optical (NLO) properties of ADP crystal at different wavelengths (355, 532, and 1064 nm) and different orientations ([001], [100], [110], I and II). The experimental data were fitted by NLO theory, to give out the two photon absorption (TPA) coefficient β 2 and the nonlinear refractive index n 2. When the light source changed from a 40 ps, 1064 nm fundamental laser to a 30 ps, 355 nm third-harmonic-generation (THG) laser, the β 2 value increased about 5 times (0.2 × 10‑2 → 1 × 10‑2 cm GW‑1), and the n 2 value increased about 1.5 times (1.5 × 10‑16 → 2.2 × 10‑16 cm2 W‑1). Among all of the orientations, the [110] sample exhibits the smallest β 2, and the second smallest n 2. It indicates that this orientation and its surroundings will be the preferred directions for high-power laser applications of ADP crystal.
All-optical image processing with nonlinear liquid crystals
Hong, Kuan-Lun
Liquid crystals are fascinating materials because of several advantages such as large optical birefringence, dielectric anisotropic, and easily compatible to most kinds of materials. Compared to the electro-optical properties of liquid crystals widely applied in displays and switching application, transparency through most parts of wavelengths also makes liquid crystals a better candidate for all-optical processing. The fast response time of liquid crystals resulting from multiple nonlinear effects, such as thermal and density effect can even make real-time processing realized. In addition, blue phase liquid crystals with spontaneously self-assembled three dimensional cubic structures attracted academic attention. In my dissertation, I will divide the whole contents into six parts. In Chapter 1, a brief introduction of liquid crystals is presented, including the current progress and the classification of liquid crystals. Anisotropy and laser induced director axis reorientation is presented in Chapter 2. In Chapter 3, I will solve the electrostrictive coupled equation and analyze the laser induced thermal and density effect in both static and dynamic ways. Furthermore, a dynamic simulation of laser induced density fluctuation is proposed by applying finite element method. In Chapter 4, two image processing setups are presented. One is the intensity inversion experiment in which intensity dependent phase modulation is the mechanism. The other is the wavelength conversion experiment in which I can read the invisible image with a visible probe beam. Both experiments are accompanied with simulations to realize the matching between the theories and practical experiment results. In Chapter 5, optical properties of blue phase liquid crystals will be introduced and discussed. The results of grating diffractions and thermal refractive index gradient are presented in this chapter. In addition, fiber arrays imaging and switching with BPLCs will be included in this chapter
Optically nonlinear energy transfer in light-harvesting dendrimers
Andrews, David L.; Bradshaw, David S.
2004-08-01
Dendrimeric polymers are the subject of intense research activity geared towards their implementation in nanodevice applications such as energy harvesting systems, organic light-emitting diodes, photosensitizers, low-threshold lasers, and quantum logic elements, etc. A recent development in this area has been the construction of dendrimers specifically designed to exhibit novel forms of optical nonlinearity, exploiting the unique properties of these materials at high levels of photon flux. Starting from a thorough treatment of the underlying theory based on the principles of molecular quantum electrodynamics, it is possible to identify and characterize several optically nonlinear mechanisms for directed energy transfer and energy pooling in multichromophore dendrimers. Such mechanisms fall into two classes: first, those where two-photon absorption by individual donors is followed by transfer of the net energy to an acceptor; second, those where the excitation of two electronically distinct but neighboring donor groups is followed by a collective migration of their energy to a suitable acceptor. Each transfer process is subject to minor dissipative losses. In this paper we describe in detail the balance of factors and the constraints that determines the favored mechanism, which include the excitation statistics, structure of the energy levels, laser coherence factors, chromophore selection rules and architecture, possibilities for the formation of delocalized excitons, spectral overlap, and the overall distribution of donors and acceptors. Furthermore, it transpires that quantum interference between different mechanisms can play an important role. Thus, as the relative importance of each mechanism determines the relevant nanophotonic characteristics, the results reported here afford the means for optimizing highly efficient light-harvesting dendrimer devices.
Nonlinear Optical Magnetism Revealed by Second-Harmonic Generation in Nanoantennas.
Kruk, Sergey S; Camacho-Morales, Rocio; Xu, Lei; Rahmani, Mohsen; Smirnova, Daria A; Wang, Lei; Tan, Hark Hoe; Jagadish, Chennupati; Neshev, Dragomir N; Kivshar, Yuri S
2017-06-14
Nonlinear effects at the nanoscale are usually associated with the enhancement of electric fields in plasmonic structures. Recently emerged new platform for nanophotonics based on high-index dielectric nanoparticles utilizes optically induced magnetic response via multipolar Mie resonances and provides novel opportunities for nanoscale nonlinear optics. Here, we observe strong second-harmonic generation from AlGaAs nanoantennas driven by both electric and magnetic resonances. We distinguish experimentally the contribution of electric and magnetic nonlinear response by analyzing the structure of polarization states of vector beams in the second-harmonic radiation. We control continuously the transition between electric and magnetic nonlinearities by tuning polarization of the optical pump. Our results provide a direct observation of nonlinear optical magnetism through selective excitation of multipolar nonlinear modes in nanoantennas.
International Nuclear Information System (INIS)
Yelin, S.F.; Hemmer, P.R.
2002-01-01
A novel class of coherent nonlinear optical phenomena, involving induced transparency in semiconductor quantum wells, is considered in the context of a particular application to sensitive long-wavelength infrared detection. It is shown that the strongest decoherence mechanisms can be suppressed or mitigated, resulting in substantial enhancement of nonlinear optical effects in semiconductor quantum wells
Performance emulation and parameter estimation for nonlinear fibre-optic links
DEFF Research Database (Denmark)
Piels, Molly; Porto da Silva, Edson; Zibar, Darko
2016-01-01
Fibre-optic communication systems, especially when operating in the nonlinear regime, generally do not perform exactly as theory would predict. A number of methods for data-based evaluation of nonlinear fibre-optic link parameters, both for accurate performance emulation and optimization...
Energy Technology Data Exchange (ETDEWEB)
Golde, Daniel
2010-06-22
In the major part of this Thesis, we discuss the linear THz response of semiconductor nanostructures based on a microscopic theory. Here, two different problems are investigated: intersubband transitions in optically excited quantum wells and the THz plasma response of two-dimensional systems. In the latter case, we analyze the response of correlated electron and electron-hole plasmas. Extracting the plasma frequency from the linear response, we find significant deviations from the commonly accepted two-dimensional plasma frequency. Besides analyzing the pure plasma response, we also consider an intermediate regime where the response of the electron-hole plasma consists of a mixture of plasma contributions and excitonic transitions. A quantitative experiment-theory comparison provides novel insights into the behavior of the system at the transition from one regime to the other. The discussion of the intersubband transitions mainly focuses on the coherent superposition of the responses from true THz transitions and the ponderomotively accelerated carriers. We present a simple method to directly identify ponderomotive effects in the linear THz response. Apart from that, the excitonic contributions to intersubband transitions are investigated. The last part of the present Thesis deals with a completely different regime. Here, the extreme nonlinear optical response of low-dimensional semiconductor structures is discussed. Formally, extreme nonlinear optics describes the regime of light-matter interaction where the exciting field is strong enough such that the Rabi frequency is comparable to or larger than the characteristic transition frequency of the investigated system. Here, the Rabi frequency is given by the product of the electrical field strength and the dipole-matrix element of the respective transition. Theoretical investigations have predicted a large number of novel nonlinear effects arising for such strong excitations. Some of them have been observed in
Khushaini, Muhammad Asif A.; Ibrahim, Abdel-Baset M. A.; Choudhury, P. K.
2018-05-01
In this paper, we provide a complete mathematical model of the phenomenon of optical bistability (OB) resulting from the degenerate two-wave mixing (TWM) process of laser beams interacting with a single nonlinear layer of ferroelectric material. Starting with the electromagnetic wave equation for optical wave propagating in nonlinear media, a nonlinear coupled wave (CW) system with both self-phase modulation (SPM) and cross-phase modulation (XPM) sources of nonlinearity are derived. The complete CW system with full nonlinearity is solved numerically and a comparison between both the cases of with and without SPM at various combinations of design parameters is given. Furthermore, to provide a reliable theoretical model for the OB via TWM process, the results obtained theoretically are compared with the available experimental data. We found that the nonlinear system without SPM fails to predict the bistable response at lower combinations of the input parameters. However, at relatively higher values, the solution without SPM shows a reduction in the switching contrast and period in the OB response. A comparison with the experimental results shows better agreement with the system with full nonlinearity.
Soliton interaction in the coupled mixed derivative nonlinear Schroedinger equations
International Nuclear Information System (INIS)
Zhang Haiqiang; Tian Bo; Lue Xing; Li He; Meng Xianghua
2009-01-01
The bright one- and two-soliton solutions of the coupled mixed derivative nonlinear Schroedinger equations in birefringent optical fibers are obtained by using the Hirota's bilinear method. The investigation on the collision dynamics of the bright vector solitons shows that there exists complete or partial energy switching in this coupled model. Such parametric energy exchanges can be effectively controlled and quantificationally measured by analyzing the collision dynamics of the bright vector solitons. The influence of two types of nonlinear coefficient parameters on the energy of each vector soliton, is also discussed. Based on the significant energy transfer between the two components of each vector soliton, it is feasible to exploit the future applications in the design of logical gates, fiber directional couplers and quantum information processors.
Exploring lipids with nonlinear optical microscopy in multiple biological systems
Alfonso-Garcia, Alba
Lipids are crucial biomolecules for the well being of humans. Altered lipid metabolism may give rise to a variety of diseases that affect organs from the cardiovascular to the central nervous system. A deeper understanding of lipid metabolic processes would spur medical research towards developing precise diagnostic tools, treatment methods, and preventive strategies for reducing the impact of lipid diseases. Lipid visualization remains a complex task because of the perturbative effect exerted by traditional biochemical assays and most fluorescence markers. Coherent Raman scattering (CRS) microscopy enables interrogation of biological samples with minimum disturbance, and is particularly well suited for label-free visualization of lipids, providing chemical specificity without compromising on spatial resolution. Hyperspectral imaging yields large datasets that benefit from tailored multivariate analysis. In this thesis, CRS microscopy was combined with Raman spectroscopy and other label-free nonlinear optical techniques to analyze lipid metabolism in multiple biological systems. We used nonlinear Raman techniques to characterize Meibum secretions in the progression of dry eye disease, where the lipid and protein contributions change in ratio and phase segregation. We employed similar tools to examine lipid droplets in mice livers aboard a spaceflight mission, which lose their retinol content contributing to the onset of nonalcoholic fatty-liver disease. We also focused on atherosclerosis, a disease that revolves around lipid-rich plaques in arterial walls. We examined the lipid content of macrophages, whose variable phenotype gives rise to contrasting healing and inflammatory activities. We also proposed new label-free markers, based on lifetime imaging, for macrophage phenotype, and to detect products of lipid oxidation. Cholesterol was also detected in hepatitis C virus infected cells, and in specific strains of age-related macular degeneration diseased cells by
Laboratory beam-plasma interactions linear and nonlinear
International Nuclear Information System (INIS)
Christiansen, P.J.; Bond, J.W.; Jain, V.K.
1982-01-01
This chapter attempts to demonstrate that despite unavoidable scaling limitations, laboratory experiments can uncover details of beam plasma interaction processes which could never be revealed through space plasma physics. Topics covered include linear theory, low frequency couplings, indirect effects, nonlinear effects, quasi-linear effects, trapping effects, nonlinear wave-wave interactions, and self modulation and cavitation. Unstable electrostatic waves arising from an exchange of energy with the ''free energy'' beam features are considered as kinetic and as hydrodynamic, or fluid, instabilities. The consequences of such instabilities (e.g. when the waves have grown to a finite level) are examined and some studies are reviewed which have attempted to understand how the free energy originally available in the beam is redistributed to produce a final state of equilibrium turbulence
Evaluation of third order nonlinear optical parameters of CdS/PVA nanocomposite
International Nuclear Information System (INIS)
Sharma, Mamta; Tripathi, S. K.
2015-01-01
CdS nanoparticles dispersed in PVA are prepared by Chemical method at room temperature. The nonlinear optical parameters such as nonlinear absorption (β), nonlinear refractive index (n 2 ) and nonlinear susceptibility (χ 3 ) are calculated for this sample by using Z-scan technique. CdS/PVA samples show the two photon absorption mechanism. The third order nonlinear susceptibility is calculated from n 2 and β and is found to be of the order of 10 −7 – 10 −8 m 2 /V 2 . The larger value of third order nonlinear susceptibility is due to dielectric and quantum confinement effect
Yang, Y.; Solis Escalante, T.; van der Helm, F.C.T.; Schouten, A.C.
2016-01-01
Objective: This paper introduces a generalized coherence framework for detecting and characterizing nonlinear interactions in the nervous system, namely cross-spectral coherence (CSC). CSC can detect different types of nonlinear interactions including harmonic and intermodulation coupling as present
Energy Technology Data Exchange (ETDEWEB)
Chen, Hua-Jun; Zhu, Ka-Di [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, 800 DongChuan Road, Shanghai 2 00240 (China)
2013-12-07
Nanomechanical resonator makes itself as an ideal system for ultrasensitive mass sensing due to its ultralow mass and high vibrational frequency. The mass sensing principle is due to the linear relationship of the frequency-shift and mass-variation. In this work, we will propose a nonlinear optical mass sensor based on a doubly clamped suspended carbon nanotube resonator in all-optical domain. The masses of external particles (such as nitric oxide molecules) landing onto the surface of carbon nanotube can be determined directly and accurately via using the nonlinear optical spectroscopy. This mass sensing proposed here may provide a nonlinear optical measurement technique in quantum measurements and environmental science.
Nonlinear degenerate cross-diffusion systems with nonlocal interaction
Di Francesco, M.; Esposito, A.; Fagioli, S.
2017-01-01
We investigate a class of systems of partial differential equations with nonlinear cross-diffusion and nonlocal interactions, which are of interest in several contexts in social sciences, finance, biology, and real world applications. Assuming a uniform "coerciveness" assumption on the diffusion part, which allows to consider a large class of systems with degenerate cross-diffusion (i.e. of porous medium type) and relaxes sets of assumptions previously considered in the literature, we prove g...
NONLINEAR OPTICAL MOLECULAR CRYSTAL BASED ON 2,6-DIAMINOPYRIDINE: SYNTHESIS AND CHARACTERIZATION
Directory of Open Access Journals (Sweden)
I. M. Pavlovetc
2014-05-01
Full Text Available The paper deals with investigation of a new nonlinear optical material based on nonlinear optical chromophore (4-Nitrophenol and aminopyridine (2,6-Diaminopyridine. Calculation results are presented for molecular packing in the crystalline compound, based on the given components. According to these results the finite material must have a noncentrosymmetric lattice, which determines the presence of the second order nonlinear optical response. Investigations carried out in this work confirm these calculations. Results of experiments are given describing the co-crystallization of these components and the following re-crystallization of the obtained material. In order to get a monocrystal form, the optimal conditions for the synthesis of molecular crystals based on these components are determined. Sufficiently large homogeneous crystals are obtained, that gave the possibility to record their spectra in the visible and near infrared parts of the spectrum, to determine their nonlinear optical properties and the level of homogeneity. Their optical (optical transmission and optical laser damage threshold and nonlinear optical properties are presented. For observation and measurement of the nonlinear optical properties an installation was built which implements the comparative method for measurements of nonlinear optical properties. A potassium titanyl oxide phosphate crystal was used as a sample for comparison. Results are given for the conversion efficiency of the primary laser radiation in the second optical harmonic relative to the signal obtained on the potassium titanyl oxide phosphate crystal. Obtained results show that the molecular co-crystal based on 2,6-Diaminopyridine is a promising nonlinear optical material for generating the second optical harmonic on the Nd: YAG laser (532 nm.
Directory of Open Access Journals (Sweden)
El-Sayed A. El-Badawy
2008-02-01
Full Text Available Although research into the use of optics in computers has increased in the last and current decades, the fact remains that electronics is still superior to optics in almost every way. Research into the use of optics at this stage mirrors the research into electronics after the 2nd World War. The advantages of using fiber optics over wiring are the same as the argument for using optics over electronics in computers. Even through totally optical computers are now a reality, computers that combine both electronics and optics, electro-optic hybrids, have been in use for some time. In the present paper, architecture of optical interconnect is built up on the bases of four Vertical-Cavity Surface- Emitting Laser Diodes (VCSELD and two optical links where thermal effects of both the diodes and the links are included. Nonlinear relations are correlated to investigate the power-current and the voltage-current dependences of the four devices. The good performance (high speed of the interconnect is deeply and parametrically investigated under wide ranges of the affecting parameters. The high speed performance is processed through three different effects, namely the device 3-dB bandwidth, the link dispersion characteristics, and the transmitted bit rate (soliton. Eight combinations are investigated; each possesses its own characteristics. The best architecture is the one composed of VCSELD that operates at 850 nm and the silica fiber whatever the operating set of causes. This combination possesses the largest device 3-dB bandwidth, the largest link bandwidth and the largest soliton transmitted bit rate. The increase of the ambient temperature reduces the high-speed performance of the interconnect
Nonlinear dynamics of resonant electrons interacting with coherent Langmuir waves
Tobita, Miwa; Omura, Yoshiharu
2018-03-01
We study the nonlinear dynamics of resonant particles interacting with coherent waves in space plasmas. Magnetospheric plasma waves such as whistler-mode chorus, electromagnetic ion cyclotron waves, and hiss emissions contain coherent wave structures with various discrete frequencies. Although these waves are electromagnetic, their interaction with resonant particles can be approximated by equations of motion for a charged particle in a one-dimensional electrostatic wave. The equations are expressed in the form of nonlinear pendulum equations. We perform test particle simulations of electrons in an electrostatic model with Langmuir waves and a non-oscillatory electric field. We solve equations of motion and study the dynamics of particles with different values of inhomogeneity factor S defined as a ratio of the non-oscillatory electric field intensity to the wave amplitude. The simulation results demonstrate deceleration/acceleration, thermalization, and trapping of particles through resonance with a single wave, two waves, and multiple waves. For two-wave and multiple-wave cases, we describe the wave-particle interaction as either coherent or incoherent based on the probability of nonlinear trapping.
Brain plasticity and functionality explored by nonlinear optical microscopy
Sacconi, L.; Allegra, L.; Buffelli, M.; Cesare, P.; D'Angelo, E.; Gandolfi, D.; Grasselli, G.; Lotti, J.; Mapelli, J.; Strata, P.; Pavone, F. S.
2010-02-01
In combination with fluorescent protein (XFP) expression techniques, two-photon microscopy has become an indispensable tool to image cortical plasticity in living mice. In parallel to its application in imaging, multi-photon absorption has also been used as a tool for the dissection of single neurites with submicrometric precision without causing any visible collateral damage to the surrounding neuronal structures. In this work, multi-photon nanosurgery is applied to dissect single climbing fibers expressing GFP in the cerebellar cortex. The morphological consequences are then characterized with time lapse 3-dimensional two-photon imaging over a period of minutes to days after the procedure. Preliminary investigations show that the laser induced fiber dissection recalls a regenerative process in the fiber itself over a period of days. These results show the possibility of this innovative technique to investigate regenerative processes in adult brain. In parallel with imaging and manipulation technique, non-linear microscopy offers the opportunity to optically record electrical activity in intact neuronal networks. In this work, we combined the advantages of second-harmonic generation (SHG) with a random access (RA) excitation scheme to realize a new microscope (RASH) capable of optically recording fast membrane potential events occurring in a wide-field of view. The RASH microscope, in combination with bulk loading of tissue with FM4-64 dye, was used to simultaneously record electrical activity from clusters of Purkinje cells in acute cerebellar slices. Complex spikes, both synchronous and asynchronous, were optically recorded simultaneously across a given population of neurons. Spontaneous electrical activity was also monitored simultaneously in pairs of neurons, where action potentials were recorded without averaging across trials. These results show the strength of this technique in describing the temporal dynamics of neuronal assemblies, opening promising
Nonlinear optical response in a zincblende GaN cylindrical quantum dot with donor impurity center
Energy Technology Data Exchange (ETDEWEB)
Hoyos, Jaime H. [Departamento de Ciencias Básicas, Universidad de Medellín, Cra. 87 No. 30-65, Medellín (Colombia); Correa, J.D., E-mail: jcorrea@udem.edu.co [Departamento de Ciencias Básicas, Universidad de Medellín, Cra. 87 No. 30-65, Medellín (Colombia); Mora-Ramos, M.E. [Centro de Investigación en Ciencias, Instituto de Investigación en Ciencias Básicas y Aplicadas, Universidad Autónoma del Estado de Morelos, Av. Universidad 1001, CP 62209 Cuernavaca, Morelos (Mexico); Duque, C.A. [Grupo de Materia Condensada-UdeA, Instituto de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín (Colombia)
2016-03-01
We calculate the nonlinear optical absorption coefficient of a cylindrical zincblende GaN-based quantum dot. For this purpose, we consider Coulomb interactions between electrons and an impurity ionized donor atom. The electron-donor-impurity spectrum and the associated quantum states are calculated using the effective mass approximation with a parabolic potential energy model describing both the radial and axial electron confinement. We also include the effects of the hydrostatic pressure and external electrostatic fields. The energy spectrum is obtained through an expansion of the eigenstates as a linear combination of Gaussian-type functions which reduces the computational effort since all the matrix elements are obtained analytically. Therefore, the numerical problem is reduced to the direct diagonalization of the Hamiltonian. The obtained energies are used in the evaluation of the dielectric susceptibility and the nonlinear optical absorption coefficient within a modified two-level approach in a rotating wave approximation. This quantity is investigated as a function of the quantum dot dimensions, the impurity position, the external electric field intensity and the hydrostatic pressure. The results of this research could be important in the design and fabrication of zincblende GaN-quantum-dot-based electro-optical devices.
Nonlinear optical response in a zincblende GaN cylindrical quantum dot with donor impurity center
International Nuclear Information System (INIS)
Hoyos, Jaime H.; Correa, J.D.; Mora-Ramos, M.E.; Duque, C.A.
2016-01-01
We calculate the nonlinear optical absorption coefficient of a cylindrical zincblende GaN-based quantum dot. For this purpose, we consider Coulomb interactions between electrons and an impurity ionized donor atom. The electron-donor-impurity spectrum and the associated quantum states are calculated using the effective mass approximation with a parabolic potential energy model describing both the radial and axial electron confinement. We also include the effects of the hydrostatic pressure and external electrostatic fields. The energy spectrum is obtained through an expansion of the eigenstates as a linear combination of Gaussian-type functions which reduces the computational effort since all the matrix elements are obtained analytically. Therefore, the numerical problem is reduced to the direct diagonalization of the Hamiltonian. The obtained energies are used in the evaluation of the dielectric susceptibility and the nonlinear optical absorption coefficient within a modified two-level approach in a rotating wave approximation. This quantity is investigated as a function of the quantum dot dimensions, the impurity position, the external electric field intensity and the hydrostatic pressure. The results of this research could be important in the design and fabrication of zincblende GaN-quantum-dot-based electro-optical devices.
Edison, D. Joseph; Nirmala, W.; Kumar, K. Deva Arun; Valanarasu, S.; Ganesh, V.; Shkir, Mohd.; AlFaify, S.
2017-10-01
Aluminium doped (i.e. 3 at%) zinc oxide (AZO) thin films were prepared by simple successive ionic layer adsorption and reaction (SILAR) method with different dipping cycles. The structural and surface morphology of AZO thin films were studied by using X-ray diffraction (XRD) and scanning electron microscopy (SEM). The optical parameters such as, transmittance, band gap, refractive index, extinction coefficient, dielectric constant and nonlinear optical properties of AZO films were investigated. XRD pattern revealed the formation of hexagonal phase ZnO and the intensity of the film was found to increase with increasing dipping cycle. The crystallite size was found to be in the range of 29-37 nm. Scanning Electron Microscope (SEM) images show the presence of small sized grains, revealing that the smoothest surface was obtained at all the films. The EDAX spectrum of AZO conforms the presence of Zn, O and Al. The optical transmittance in the visible region is high 87% and the band gap value is 3.23 eV. The optical transmittance is decreased with respect to dipping cycles. The room temperature PL studies revealed that the AZO films prepared at (30 cycles) has good film quality with lesser defect density. The third order nonlinear optical parameters were also studied using Z-scan technique to know the applications of deposited films in nonlinear devices. The third order nonlinear susceptibility value is found to be 1.69 × 10-7, 3.34 × 10-8, 1.33 × 10-7and 2.52 × 10-7 for AZO films deposited after 15, 20, 25 and 30 dipping cycles.
Nonlinear localized modes in dipolar Bose-Einstein condensates in optical lattices
International Nuclear Information System (INIS)
Rojas-Rojas, S.; Vicencio, R. A.; Molina, M. I.; Abdullaev, F. Kh.
2011-01-01
Modulational instability and discrete matter wave solitons in dipolar BECs, loaded into a deep optical lattice, are investigated analytically and numerically. The process of modulational instability of nonlinear plane matter waves in a dipolar nonlinear lattice is studied and the regions of instability are established. The existence and stability of bulk discrete solitons are analyzed analytically and confirmed by numerical simulations. In marked contrast with the usual discrete nonlinear Schroedinger behavior (no dipolar interactions), we found a region where the two fundamental modes are simultaneously unstable, allowing enhanced mobility across the lattice for large norm values. To study the existence and properties of surface discrete solitons, an analysis of the dimer configuration is performed. The properties of symmetric and antisymmetric modes including stability diagrams and bifurcations are investigated in closed form. For the case of a bulk medium, properties of fundamental on-site and intersite localized modes are analyzed. On-site and intersite surface localized modes are studied, and we find that they do not exist when nonlocal interactions predominate with respect to local ones.
International Nuclear Information System (INIS)
Feng Miao; Zhan Hongbing; Sun Ruiqing; Chen Yu
2010-01-01
The implantation and growth of metal nanoparticles on graphene nanosheets (GNS) leads directly to severe damage to the regular structure of the graphene sheets, which disrupts the extended π conjugation, resulting in an impaired device performance. In this paper, we describe a facile approach for achieving the lossless formation of graphene composite decorated with tiny cadmium sulfide quantum dots (QDs) with excellent nonlinear optical properties by using benzyl mercaptan (BM) as the interlinker. The mercapto substituent of BM binds to the CdS QDs during their nucleation and growth process, and then the phenyl comes into contact with the GNS via the π-π stacking interaction. Using this strategy, CdS QDs with an average diameter of 3 nm are uniformly dispersed over the surface of graphene, and the resulting QD-graphene composite exhibits excellent optical limiting properties, mainly contributed by nonlinear scattering and nonlinear absorption, upon both 532 and 1064 nm excitations, in the nanosecond laser pulse regime.
Nonlinear optical switching behavior in the solid state: A theoretical investigation on anils
Ségerie, Audrey
2011-09-13
The linear (π(1)) and second-order nonlinear (π(2)) optical properties of two anil crystals, [N-(4-hydroxy)-salicylidene-amino-4-(methylbenzoate) and N-(3,5-di-tert- butylsalicylidene)-4-aminopyridine, denoted 4A and 4P, respectively], as well as the optical contrasts upon switching between their enol (E) and keto (K) forms, have been investigated by combining the molecular responses calculated using quantum chemistry methods and an electrostatic interaction scheme to account for the local field effects. It is found that intermolecular interactions impact differently the K/E optical contrasts in the two systems, which illustrates the importance of the supramolecular organization on the macroscopic responses. In 4A, the surrounding effects on the (hyper)polarizabilities are similar in the enol and keto forms, leading to optical contrasts very close to those of the isolated molecule. In contrast, an enhancement of the second-order susceptibility is observed in the keto form of 4P, leading to a large π(2)(K)/π(2)(E) contrast. Moreover, the π(2)(4A)/π(2)(4P) ratio for the most stable enol forms is obtained to be in good agreement with previous experimental investigations, which supports the reliability of the computational procedure. © 2011 American Chemical Society.
Nonlinear optical switching behavior in the solid state: A theoretical investigation on anils
Sé gerie, Audrey; Castet, Fré dé ric; Kanoun, Mohammed; Plaquet, Auré lie; Lié geois, Vincent; Champagne, Benoit
2011-01-01
The linear (π(1)) and second-order nonlinear (π(2)) optical properties of two anil crystals, [N-(4-hydroxy)-salicylidene-amino-4-(methylbenzoate) and N-(3,5-di-tert- butylsalicylidene)-4-aminopyridine, denoted 4A and 4P, respectively], as well as the optical contrasts upon switching between their enol (E) and keto (K) forms, have been investigated by combining the molecular responses calculated using quantum chemistry methods and an electrostatic interaction scheme to account for the local field effects. It is found that intermolecular interactions impact differently the K/E optical contrasts in the two systems, which illustrates the importance of the supramolecular organization on the macroscopic responses. In 4A, the surrounding effects on the (hyper)polarizabilities are similar in the enol and keto forms, leading to optical contrasts very close to those of the isolated molecule. In contrast, an enhancement of the second-order susceptibility is observed in the keto form of 4P, leading to a large π(2)(K)/π(2)(E) contrast. Moreover, the π(2)(4A)/π(2)(4P) ratio for the most stable enol forms is obtained to be in good agreement with previous experimental investigations, which supports the reliability of the computational procedure. © 2011 American Chemical Society.
Thangaraj, M.; Vinitha, G.; Sabari Girisun, T. C.; Anandan, P.; Ravi, G.
2015-10-01
Optical nonlinearity of metal complexes of p-nitrophenolate (M=Li, Na and K) in ethanol is studied by using a continuous wave (cw) diode pumped Nd:YAG laser (532 nm, 50 mW). The predominant mechanism of observed nonlinearity is thermal in origin. The nonlinear refractive index and the nonlinear absorption coefficient of the samples were found to be in the order of 10-8 cm2/W and 10-3 cm/W respectively. Magnitude of third-order optical parameters varies according to the choice of alkali metal chosen for metal complex formation of p-nitrophenolate. The third-order nonlinear susceptibility was found to be in the order of 10-6 esu. The observed saturable absorption and the self-defocusing effect were used to demonstrate the optical limiting action at 532 nm by using the same cw laser beam.
Pramodini, S.; Sudhakar, Y. N.; SelvaKumar, M.; Poornesh, P.
2014-04-01
We present the synthesis and characterization of third-order optical nonlinearity and optical limiting of the conducting polymers poly (aniline-co-o-anisidine) and poly (aniline-co-pyrrole). Nonlinear optical studies were carried out by employing the z-scan technique using a He-Ne laser operating in continuous wave mode at 633 nm. The copolymers exhibited a reverse saturable absorption process and self-defocusing properties under the experimental conditions. The estimated values of βeff, n2 and χ(3) were found to be of the order of 10-2 cm W-1, 10-5 esu and 10-7 esu respectively. Self-diffraction rings were observed due to refractive index change when exposed to the laser beam. The copolymers possess a lower limiting threshold and clamping level, which is essential to a great extent for power limiting devices. Therefore, copolymers of aniline emerge as a potential candidate for nonlinear optical device applications.
DEFF Research Database (Denmark)
Webb, Garry; Sørensen, Mads Peter; Brio, Moysey
2004-01-01
the electromagnetic momentum and energy conservation laws, corresponding to the space and time translation invariance symmetries. The symmetries are used to obtain classical similarity solutions of the equations. The traveling wave similarity solutions for the case of a cubic Kerr nonlinearity, are shown to reduce...... the properties of Maxwell's equations in nonlinear optics, without resorting to the commonly used nonlinear Schr\\"odinger (NLS) equation approximation in which a high frequency carrier wave is modulated on long length and time scales due to nonlinear sideband wave interactions. This is important in femto......-second pulse propagation in which the NLS approximation is expected to break down. The canonical Hamiltonian description of the equations involves the solution of a polynomial equation for the electric field $E$, in terms of the the canonical variables, with possible multiple real roots for $E$. In order...
Homogenous smooth sol gel films doped with organic compounds for nonlinear optics
Energy Technology Data Exchange (ETDEWEB)
Vasiliu, I.C. [INOE 2000 — National Institute for Optoelectronics, 409 Atomistilor Str., Magurele, Bucharest, RO 077125 (Romania); Ionita, I., E-mail: i_ionita@yahoo.com [UB — University of Bucharest, 405 Atomistilor Str., Magurele, Bucharest, RO 077125 (Romania); Matei, A. [INFLPR — National Institute for Laser, Plasma and Radiation Physics, 409 Atomistilor Str., Magurele, Bucharest, RO 077125 (Romania); Elisa, M.; Iordanescu, R.; Feraru, I.; Emandi, A. [INOE 2000 — National Institute for Optoelectronics, 409 Atomistilor Str., Magurele, Bucharest, RO 077125 (Romania)
2016-02-29
The demand for protection of various types of optical sensors from laser-beam pulses has resulted in the search for optical limiting devices that have the property of being transparent at low intensity of light (normal light), but no transparent towards high intensity (laser) light. Organic material with nonlinear optical (NLO) properties as reverse saturable absorption and two-photon absorption can be used for optical limiting with the advantage of a very fast response and self-activation. A promising approach in the fabrication of thin films by low cost/easy use deposition methods for second-order nonlinear optics is sol–gel technique. The present paper reports on the sol–gel synthesis of some pyrazolone derivative doped SiO{sub 2}–P{sub 2}O{sub 5} smooth and homogenous films (Root mean square roughness (Rq) = 1.1 nm) using as precursors tetraethylorthosilicate (TEOS) and phosphoric acid (H{sub 3}PO{sub 4}). The structure of the deposited azo-derivatives doped thin films was examined by Fourier transform infrared spectroscopy and atomic force microscopy, while their optical properties of the films by UV–VIS spectroscopy. The nonlinear optical efficiencies due to the interaction of the NLO-active chromophores with the inorganic matrix have a significant influence on the second harmonic generation capabilities that was measured using a femtosecond Ti:Sapphire laser. The properties of the films were investigated and correlated with the concentration of the organic dopant and the thermal treatment temperature. - Highlights: • We obtained pyrazolone derivative doped SiO{sub 2}–P{sub 2}O{sub 5} smooth and homogenous films. • The pyrazolone derivative presents SHG characteristics by itself. • Thin sol gel films doped with organic compounds with NLO properties. • Temperature of thermal treatment and aging time can improve NLO properties of films. • We found that 150 °C and 28 h aging time give the maximum performance in SHG response.
Optical Lattice Gases of Interacting Fermions
2015-12-02
interacting Fermi gases has topological properties similar to the conventional chiral p- wave state. These include a non-zero Chern number and the...interacting cold gases with broad impacts on the interfaces with condensed matter and particle physics . Applications and experiments of some of the physics ...AFRL-AFOSR-VA-TR-2016-0016 Optical Lattice Gases of Interacting Fermions Wensheng Vincent Liu UNIVERSITY OF PITTSBURGH Final Report 12/02/2015
Nonlinear optical control of Josephson coupling in cuprates
Energy Technology Data Exchange (ETDEWEB)
Casandruc, Eliza
2017-03-15
In High-T{sub C} cuprates superconducting Cu-O planes alternate with insulating layers along the crystallographic c-axis, making the materials equivalent to Josephson junctions connected in series. The most intriguing consequence is that the out-of-plane superconducting transport occurs via Cooper pairs tunneling across the insulating layers and can be predicted by the Josephson tunneling equations. Nonlinear interaction between light fields and the superconducting carriers serves as a powerful dynamical probe of cuprates, while offering opportunities for controlling them in an analogous fashion to other stimuli such as pressure and magnetic fields. The main goal of this thesis work is to use intense transient light fields to control the interlayer superconducting transport on ultrafast time scales. This was achieved by tuning the wavelength of such light pulses to completely different ranges, in order to either directly excite Josephson Plasma Waves in the nonlinear regime, or efficiently melt the competing charge and spin order phase, which in certain cuprates quenches the Josephson tunneling at equilibrium. In a first study, I have utilized strong field terahertz transients with frequencies tuned to the Josephson plasma resonance (JPR) to coherently control the c-axis superconducting transport. The Josephson relations have a cubic nonlinearity which is exploited to achieve two related, albeit slightly different, phenomena. Depending on the driving pulse, solitonic breathers were excited with narrow-band multi-cycle pulses in La{sub 1.84}Sr{sub 0.16}CuO{sub 4} while broad-band half-cycle pulses were employed to achieve a parametric amplification of Josephson Plasma Waves in La{sub 1.905}Ba{sub 0.095}CuO{sub 4}. These experiments are supported by extensive modeling, showing exceptional agreement. A comprehensive study illustrates the strong enhancement of the nonlinear effects near the JPR frequency. Then, I turned to investigate the competition between
An, Hong-Lin; Arriola, Alexander; Gross, Simon; Fuerbach, Alexander; Withford, Michael J.; Fleming, Simon
2014-01-01
The thermal poling technique was applied to optical waveguides embedded in a commercial boro-aluminosilicate glass, resulting in high levels of induced second-order optical nonlinearity. The waveguides were fabricated using the femtosecond laser direct-write technique, and thermally poled samples were characterized with second harmonic optical microscopy to reveal the distribution profile of the induced nonlinearity. It was found that, in contrast to fused silica, the presence of waveguides in boro-aluminosilicate glass led to an enhancement of the creation of the second-order nonlinearity, which is larger in the laser written waveguiding regions when compared to the un-modified substrate. The magnitude of the nonlinear coefficient d33 achieved in the core of the laser-written waveguides, up to 0.2 pm/V, was comparable to that in thermally poled fused silica, enabling the realization of compact integrated electro-optic devices in boro-aluminosilicate glasses.
MECHANISM OF OPTICAL NONLINEARITY IN “LYOTROPIC LIQUID CRYSTAL — VIOLOGEN” SYSTEM
Directory of Open Access Journals (Sweden)
Hanna Bordyuh
2014-06-01
Full Text Available In the present work we analyze the characteristics of holographic grating recording and consider a mechanism of optical nonlinearity in the lyotropic liquid crystal (LLC — viologen samples. Taking into account structural and electrooptical properties of the admixture molecules it is possible to suggest that the recording is realized due to the change of polarizability of π-electron system of coloured viologen derivatives under the action of laser radiation. The main nonlinear optical parameters such as nonlinear refraction coefficient n2, cubic nonlinear susceptibility χ(3, and hyperpolarizability γ were calculated.
Fluid transport due to nonlinear fluid-structure interaction
DEFF Research Database (Denmark)
Jensen, Jakob Søndergaard
1997-01-01
This work considers nonlinear fluid-structure interaction for a vibrating pipe containing fluid. Transverse pipe vibrations will force the fluid to move relative to the pipe creating unidirectional fluid flow towards the pipe end. The fluid flow induced affects the damping and the stiffness...... of the pipe. The behavior of the system in response to lateral resonant base excitation is analysed numerically and by the use of a perturbation method (multiple scales). Exciting the pipe in the fundamental mode of vibration seems to be most effective for transferring energy from the shaker to the fluid......, whereas higher modes of vibration can be used to transport fluid with pipe vibrations of smaller amplitude. The effect of the nonlinear geometrical terms is analysed and these terms are shown to affect the response for higher modes of vibration. Experimental investigations show good agreement...
Third-order nonlinear optical studies of anthraquinone dyes using a CW He–Ne laser
International Nuclear Information System (INIS)
Pramodini, S; Poornesh, P
2014-01-01
We present investigations on the third-order optical nonlinearity and optical power limiting of anthraquinone dyes. Z-scan measurements were performed using a continuous wave He–Ne laser at 633 nm wavelength as an excitation source. The nonlinear refraction studies exhibited self-defocusing behavior of the dyes. The nonlinear absorption in the dyes was dominated by a reverse saturable absorption process. Self-diffraction ring patterns were observed due to the change in refractive index and thermal lensing. Increase of the electron donating ability of the substituents resulted in enhanced values of the nonlinear optical parameters, establishing the structure–property relationship. The optical limiting study revealed that the dyes possess a lower limiting threshold and clamping level which is very important for eye and sensor protection. Hence, the dyes investigated here emerge as promising candidates for future opto-electronic and photonic device applications such as optical power limiters. (paper)
Third-order nonlinear optical studies of anthraquinone dyes using a CW He-Ne laser
Pramodini, S.; Poornesh, P.
2014-05-01
We present investigations on the third-order optical nonlinearity and optical power limiting of anthraquinone dyes. Z-scan measurements were performed using a continuous wave He-Ne laser at 633 nm wavelength as an excitation source. The nonlinear refraction studies exhibited self-defocusing behavior of the dyes. The nonlinear absorption in the dyes was dominated by a reverse saturable absorption process. Self-diffraction ring patterns were observed due to the change in refractive index and thermal lensing. Increase of the electron donating ability of the substituents resulted in enhanced values of the nonlinear optical parameters, establishing the structure-property relationship. The optical limiting study revealed that the dyes possess a lower limiting threshold and clamping level which is very important for eye and sensor protection. Hence, the dyes investigated here emerge as promising candidates for future opto-electronic and photonic device applications such as optical power limiters.
Design considerations for multi component molecular-polymeric nonlinear optical materials
Energy Technology Data Exchange (ETDEWEB)
Singer, K.D. (Case Western Reserve Univ., Cleveland, OH (USA). Dept. of Physics); Kuzyk, M.G. (Washington State Univ., Pullman, WA (USA). Dept. of Physics); Fang, T.; Holland, W.R. (AT and T Bell Labs., Princeton, NJ (USA)); Cahill, P.A. (Sandia National Labs., Albuquerque, NM (USA))
1990-01-01
We review our work on multi component polymeric nonlinear optical materials. These materials consist of nonlinear optical molecules incorporated in a polymeric host. A cross-linked triazine polymer incorporating a dicyanovinyl terminated azo dye was found to be relatively stable at 85{degree} and posses an electro-optic coefficient of 11pm/V. We have also observed the zero dispersion condition in a new anomalous dispersion dye for phase matched second harmonic generation, and expect efficient conversion to the blue. A squarylium dye, ISQ, has been found to posses a large third order nonlinearity, and may display two-level behavior. 24 refs., 11 figs.
Automated seeding-based nuclei segmentation in nonlinear optical microscopy.
Medyukhina, Anna; Meyer, Tobias; Heuke, Sandro; Vogler, Nadine; Dietzek, Benjamin; Popp, Jürgen
2013-10-01
Nonlinear optical (NLO) microscopy based, e.g., on coherent anti-Stokes Raman scattering (CARS) or two-photon-excited fluorescence (TPEF) is a fast label-free imaging technique, with a great potential for biomedical applications. However, NLO microscopy as a diagnostic tool is still in its infancy; there is a lack of robust and durable nuclei segmentation methods capable of accurate image processing in cases of variable image contrast, nuclear density, and type of investigated tissue. Nonetheless, such algorithms specifically adapted to NLO microscopy present one prerequisite for the technology to be routinely used, e.g., in pathology or intraoperatively for surgical guidance. In this paper, we compare the applicability of different seeding and boundary detection methods to NLO microscopic images in order to develop an optimal seeding-based approach capable of accurate segmentation of both TPEF and CARS images. Among different methods, the Laplacian of Gaussian filter showed the best accuracy for the seeding of the image, while a modified seeded watershed segmentation was the most accurate in the task of boundary detection. The resulting combination of these methods followed by the verification of the detected nuclei performs high average sensitivity and specificity when applied to various types of NLO microscopy images.
Thermally Stable Heterocyclic Imines as New Potential Nonlinear Optical Materials
Nesterov, Volodymyr V.; Antipin, Mikhail Y.; Nesterov, Vladimir N.; Moore, Craig E.; Cardelino, Beatriz H.; Timofeeva, Tatiana V.
2004-01-01
In the course of a search for new thermostable acentric nonlinear optical crystalline materials, several heterocyclic imine derivatives were designed, with the general structure D-pi-A(D'). Introduction of a donor amino group (D') into the acceptor moiety was expected to bring H-bonds into their crystal structures, and so to elevate their melting points and assist in an acentric molecular packing. Six heterocycle-containing compounds of this type were prepared, single crystals were grown for five of them, and these crystals were characterized by X-ray analysis. A significant melting temperature elevation was found for all of the synthesized compounds. Three of the compounds were also found to crystallize in acentric space groups. One of the acentric compounds is built as a three-dimensional H-bonded molecular network. In the other two compounds, with very similar molecular structure, the molecules form one-dimensional H-bonded head-to-head associates (chains). These chains are parallel in two different crystallographic directions and form very unusual interpenetrating chain patterns in an acentric crystal. Two of the compounds crystallized with centrosymmetric molecular packing.
Nonlinear optical properties of Sn+ ion-implanted silica glass
International Nuclear Information System (INIS)
Takeda, Y.; Hioki, T.; Motohiro, T.; Noda, S.; Kurauchi, T.
1994-01-01
The absolute value of the third-order nonlinear optical susceptibility, vertical stroke χ (3) vertical stroke , of Sn + ion-implanted silica glass was found to be similar 10 -6 esu. This value is as large as those reported for semiconductor-doped glasses. Silica glass substrates were implanted with Sn + ions at an acceleration energy of 400 keV to a dose of 2x10 17 ions/cm 2 at room temperature. Metallic Sn microcrystallites of 4-20 nm in diameter were found to be embedded in the silica glass matrix. The average volume fraction of the Sn microcrystallites was evaluated to be 28%. vertical stroke χ (3) vertical stroke and the imaginary part of the dielectric function, Im ε, had peaks at the same wavelength of 500 nm owing to surface plasmon resonance. The peak width of vertical stroke χ (3) vertical stroke was nearly half of that of Im ε, which can be explained by an effective medium theory. ((orig.))
Second-Order Nonlinear Optical Dendrimers and Dendronized Hyperbranched Polymers.
Tang, Runli; Li, Zhen
2017-01-01
Second-order nonlinear optical (NLO) dendrimers with a special topological structure were regarded as the most promising candidates for practical applications in the field of optoelectronic materials. Dendronized hyperbranched polymers (DHPs), a new type of polymers with dendritic structures, proposed and named by us recently, demonstrated interesting properties and some advantages over other polymers. Some of our work concerning these two types of polymers are presented herein, especially focusing on the design idea and structure-property relationship. To enhance their comprehensive NLO performance, dendrimers were designed and synthesized by adjusting their isolation mode, increasing the number of the dendritic generation, modifying their topological structure, introducing isolation chromophores, and utilizing the Ar-Ar F self-assembly effect. To make full use of the advantages of both the structural integrity of dendrimers and the convenient one-pot synthesis of hyperbranched polymers, DHPs were explored by utilizing low-generation dendrons as big monomers to construct hyperbranched polymers. These selected works could provide valuable information to deeply understand the relationship between the structure and properties of functional polymers with dendritic structures, but not only limited to the NLO ones, and might contribute much to the further development of functional polymers with rational design. © 2017 The Chemical Society of Japan & Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.
Analysis of nonlinear optical properties in donor–acceptor materials
Energy Technology Data Exchange (ETDEWEB)
Day, Paul N. [Air Force Research Laboratory, Wright-Patterson Air Force Base, Ohio 45433 (United States); General Dynamics Information Technology, Inc., Dayton, Ohio 45431 (United States); Pachter, Ruth [Air Force Research Laboratory, Wright-Patterson Air Force Base, Ohio 45433 (United States); Nguyen, Kiet A. [Air Force Research Laboratory, Wright-Patterson Air Force Base, Ohio 45433 (United States); UES, Inc., Dayton, Ohio 45432 (United States)
2014-05-14
Time-dependent density functional theory has been used to calculate nonlinear optical (NLO) properties, including the first and second hyperpolarizabilities as well as the two-photon absorption cross-section, for the donor-acceptor molecules p-nitroaniline and dimethylamino nitrostilbene, and for respective materials attached to a gold dimer. The CAMB3LYP, B3LYP, PBE0, and PBE exchange-correlation functionals all had fair but variable performance when compared to higher-level theory and to experiment. The CAMB3LYP functional had the best performance on these compounds of the functionals tested. However, our comprehensive analysis has shown that quantitative prediction of hyperpolarizabilities is still a challenge, hampered by inadequate functionals, basis sets, and solvation models, requiring further experimental characterization. Attachment of the Au{sub 2}S group to molecules already known for their relatively large NLO properties was found to further enhance the response. While our calculations show a modest enhancement for the first hyperpolarizability, the enhancement of the second hyperpolarizability is predicted to be more than an order of magnitude.
International Nuclear Information System (INIS)
Duque, C.A.; Kasapoglu, E.; Sakiroglu, S.; Sari, H.; Soekmen, I.
2011-01-01
In this work the effects of intense laser on the electron-related nonlinear optical absorption and nonlinear optical rectification in GaAs-Ga 1-x Al x As quantum wells are studied under, applied electric and magnetic field. The electric field is applied along the growth direction of the quantum well whereas the magnetic field has been considered to be in-plane. The calculations were performed within the density matrix formalism with the use of the effective mass and parabolic band approximations. The intense laser effects are included through the Floquet method, by modifying the confining potential associated to the heterostructure. Results are presented for the nonlinear optical absorption, the nonlinear optical rectification and the resonant peak of these two optical processes. Several configurations of the dimensions of the quantum well, the applied electric and magnetic fields, and the incident intense laser radiation have been considered. The outcome of the calculation suggests that the nonlinear optical absorption and optical rectification are non-monotonic functions of the dimensions of the heterostructure and of the external perturbations considered in this work.
Kinematics of Nonlinearly Interacting MHD Instabilities in a Plasma
International Nuclear Information System (INIS)
Hansen, Alexander K.
2000-01-01
Plasmas play host to a wide variety of instabilities. For example, tearing instabilities use finite plasma resistivity to exploit the free energy provided by plasma currents parallel to the magnetic field to alter the magnetic topology of the plasma through a process known as reconnection. These instabilities frequently make themselves known in magnetic confinement experiments such as tokamaks and reversed field pinches (RFPs). In RFP plasmas, in fact, several tearing instabilities (modes) are simultaneously active, and are of large amplitude. Theory predicts that in addition to interacting linearly with magnetic perturbations from outside the plasma, such as field errors or as resistive wall, the modes in the RFP can interact nonlinearly with each other through a three-wave interaction. In the current work investigations of both the linear (external) and nonlinear contributions to the kinematics of the tearing modes in the Madison Symmetric Torus (MST) RFP are reported Theory predicts that tearing modes will respond only to magnetic perturbations that are spatially resonant with them, and was supported by experimental work done on tokamak devices. The results in this work verified that the theory is still applicable to the RFP, in spite of its more complicated magnetic mode structure, involving perturbations of a single poloidal mode number
Nonlinear instability and chaos in plasma wave-wave interactions
International Nuclear Information System (INIS)
Kueny, C.S.
1993-01-01
Conventional linear stability analysis may fail for fluid systems with an indefinite free energy functional. When such a system is linearly stable, it is said to possess negative energy modes. Instability may then occur either via dissipation of the negative energy modes. Instability may then occur either via dissipation of the negative energy modes. Instability may then occur either via dissipitation of the negative energy modes, or nonlinearly via resonant wave-wave coupling, which leads to explosive growth. In the dissipationaless case, it is conjectured that intrinsic chaotic behavior may allow initially non-resonant systems to reach resonance by diffusion in phase space. This is illustrated for a simple equilibrium involving cold counter-streaming ions. The system is described in the fluid approximation by a Hamilitonian functional and associated noncanonical Poisson bracket. By Fourier decomposition and appropriate coordinate transformations, the Hamilitonian for the perturbed energy is expressed in action-angle form. The normal modes correspond to Doppler-shifted ion-acoustic waves of positive and negative energy. Nonlinear coupling leads to decay instability via two-wave interactions, which occur generically for long enough wavelengths. Three-wave interactions which occur in isolated, but numerous, regions of parameter space can drive either decay instability or explosive instability. When the resonance for explosive growth is detuned, a stable region exists around the equilibrium point in phase space, while explosive growth occurs outside of a separatrix. These interactions may be described exactly if only one resonance is considered, while multiple nonlinear terms make the Hamiltonian nonintegradable. Simple Hamiltonians of two and three degrees of freedom are studied numerically using symplectic integration algorithms, including an explicit algorithm derived using Lie algebraic methods
Nonlinear wave particle interaction in the Earth's foreshock
Mazelle, C.; LeQueau, D.; Meziane, K.; Lin, R. P.; Parks, G.; Reme, H.; Sanderson, T.; Lepping, R. P.
1997-01-01
The possibility that ion beams could provide a free energy source for driving an ion/ion instability responsible for the ULF wave occurrence is investigated. For this, the wave dispersion relation with the observed parameters is solved. Secondly, it is shown that the ring-like distributions could then be produced by a coherent nonlinear wave-particle interaction. It tends to trap the ions into narrow cells in velocity space centered around a well-defined pitch-angle, directly related to the saturation wave amplitude in the analytical theory. The theoretical predictions with the observations are compared.
Non-linear effective Lagrangian treatment of 'Penguin' interaction
International Nuclear Information System (INIS)
Pham, T.N.
1984-01-01
Using the non-linear effective lagrangian technique, we show explicitly that only derivative coupling is allowed for the K - π, K -> 2 π and K -> 3 π transitions induced by the ΔS = 1 Penguin operator of SVZ in agreement with chiral symmetry requirements. From a derivative coupling (3, anti 3) mass term and the SU(3) breaking effect for fsub(K)/fsub(π), we estimate the strength of the Penguin interactions and find it too small to account for the ΔI = 1/2 amplitude. (orig.)
Directory of Open Access Journals (Sweden)
Nam Lyong Kang
2013-07-01
Full Text Available The projection-reduction method introduced by the present authors is known to give a validated theory for optical transitions in the systems of electrons interacting with phonons. In this work, using this method, we derive the linear and first order nonlinear optical conductivites for an electron-impurity system and examine whether the expressions faithfully satisfy the quantum mechanical philosophy, in the same way as for the electron-phonon systems. The result shows that the Fermi distribution function for electrons, energy denominators, and electron-impurity coupling factors are contained properly in organized manners along with absorption of photons for each electron transition process in the final expressions. Furthermore, the result is shown to be represented properly by schematic diagrams, as in the formulation of electron-phonon interaction. Therefore, in conclusion, we claim that this method can be applied in modeling optical transitions of electrons interacting with both impurities and phonons.
Directory of Open Access Journals (Sweden)
Shahriari
2017-02-01
Full Text Available In this work, the optical properties dependence of Multi-Walled Carbon Nanotubes (MWNT on concentration was discussed. MWNT samples were prepared in polypyrrole by an electrochemical polymerization of monomers, in the presence of different concentrations of MWNTs, using Sodium Dodecyl-Benzen-Sulfonate (SDBS as surfactant at room temperature. The nonlinear refractive and nonlinear absorbtion indices were measured using a low power CW laser beam operated at 532 nm using z-scan method. The results show that nonlinear refractive and nonlinear absorbtion indices tend to be increased with increasing the concentration of carbon nanotubes. Optical properties of carbone nanotubes indicate that they are good candidates for nonlinear optical devices
Rapid assessment of nonlinear optical propagation effects in dielectrics
Hoyo, J. Del; de La Cruz, A. Ruiz; Grace, E.; Ferrer, A.; Siegel, J.; Pasquazi, A.; Assanto, G.; Solis, J.
2015-01-01
Ultrafast laser processing applications need fast approaches to assess the nonlinear propagation of the laser beam in order to predict the optimal range of processing parameters in a wide variety of cases. We develop here a method based on the simple monitoring of the nonlinear beam shaping against numerical prediction. The numerical code solves the nonlinear Schrödinger equation with nonlinear absorption under simplified conditions by employing a state-of-the art computationally efficient approach. By comparing with experimental results we can rapidly estimate the nonlinear refractive index and nonlinear absorption coefficients of the material. The validity of this approach has been tested in a variety of experiments where nonlinearities play a key role, like spatial soliton shaping or fs-laser waveguide writing. The approach provides excellent results for propagated power densities for which free carrier generation effects can be neglected. Above such a threshold, the peculiarities of the nonlinear propagation of elliptical beams enable acquiring an instantaneous picture of the deposition of energy inside the material realistic enough to estimate the effective nonlinear refractive index and nonlinear absorption coefficients that can be used for predicting the spatial distribution of energy deposition inside the material and controlling the beam in the writing process.
Non-linear optical techniques and optical properties of condensed molecular systems
Citroni, Margherita
2013-06-01
Structure, dynamics, and optical properties of molecular systems can be largely modified by the applied pressure, with remarkable consequences on their chemical stability. Several examples of selective reactions yielding technologically attractive products can be cited, which are particularly efficient when photochemical effects are exploited in conjunction with the structural conditions attained at high density. Non-linear optical techniques are a basic tool to unveil key aspects of the chemical reactivity and dynamic properties of molecules. Their application to high-pressure samples is experimentally challenging, mainly because of the small sample dimensions and of the non-linear effects generated in the anvil materials. In this talk I will present results on the electronic spectra of several aromatic crystals obtained through two-photon induced fluorescence and two-photon excitation profiles measured as a function of pressure (typically up to about 25 GPa), and discuss the relationship between the pressure-induced modifications of the electronic structure and the chemical reactivity at high pressure. I will also present the first successful pump-probe infrared measurement performed as a function of pressure on a condensed molecular system. The system under examination is liquid water, in a sapphire anvil cell, up to 1 GPa along isotherms at 298 and 363 K. These measurements give a new enlightening insight into the dynamical properties of low- and high-density water allowing a definition of the two structures.
CHEF: an Interactive program for accelerator optics
International Nuclear Information System (INIS)
Michelotti, Leo; Ostiguy, Jean-Francois
2005-01-01
We report the current status and our plans for the completion of CHEF, an interactive application for performing optics calculations in accelerator physics. CHEF uses high level graphical user interfaces to facilitate the exploitation of lower level tools incorporated into a hierarchy of C++ class libraries, making them usable by those not familiar with C++ programming
International Nuclear Information System (INIS)
Xiao Li; Zhang Wei; Huang Yidong; Peng Jiangde
2008-01-01
High nonlinear microstructure fibre (HNMF) is preferred in nonlinear fibre optics, especially in the applications of optical parametric effects, due to its high optical nonlinear coefficient. However, polarization dependent dispersion will impact the nonlinear optical parametric process in HNMFs. In this paper, modulation instability (MI) method is used to measure the polarization dependent dispersion of a piece of commercial HNMF, including the group velocity dispersion, the dispersion slope, the fourth-order dispersion and group birefringence. It also experimentally demonstrates the impact of the polarization dependent dispersion on the continuous wave supercontinuum (SC) generation. On one axis MI sidebands with symmetric frequency detunings are generated, while on the other axis with larger MI frequency detuning, SC is generated by soliton self-frequency shift
Computational Study of Chalcopyrite Semiconductors and Their Non-Linear Optical Properties
National Research Council Canada - National Science Library
Lambrecht, Walter R
2007-01-01
... (Including cation antisites, cation and anion vacancies) and CdGeAs2; a study of the feasibility of nonciritical phase matching and associated nonlinear optical parameters in CdSiP2 and CdSIAs2...
Self-Assembly of Nanocomposite Nonlinear Optical Materials for Photonic Devices, Phase I
National Aeronautics and Space Administration — This program targets the development of new highly anisotropic nonlinear optical nanocomposite materials for NASA and non-NASA applications in advanced photonic and...
Earthquake analysis with nonlinear soil-structure interaction and nonlinear supports of components
International Nuclear Information System (INIS)
Hansson, V.
1990-01-01
For the determination of the seismic response of a structure the soil-structure interaction in most cases is modelled by a mass-spring-damper-system. Normally design concepts for components and piping are based on linear calculations and stress limitations. A concept for a reactor building for the HTR 100 consisted of a relatively high structure compared with the dimensions of the foundation. The structure was comparatively deep embedded in the soil, so here the embedment influences significantly the soil-structure interaction. The assembly of reactor vessel, heat exchanger and circulators has a height of about 37 m. Supports are arranged at different levels. Due to temperature deformations of the vessel and of the support constructions small gaps at the supports may only be avoided by complicated constructions of the supports. Nonlinear analyses were performed for soil, building and component with all supports. The finite element analyses used time histories. In order to describe the radiation damping the hysteresis of the soil with 1 percent material damping was considered. Nonlinearities in the interface of soil and foundation and due to gaps and friction at the supports were taken into account. The stiffness of the support constructions influences reactions and accelerations to a high extent. Properly chosen stiffnesses of the support constructions lead to a behaviour similar to linear elastic behaviour. 13 figs
R. Vlokh; M. Kostyrko
2006-01-01
Nonlinear effect of the gravitation field of spherically symmetric mass on the gravitational coefficient G has been analysed. In frame of the approaches of parametric optics and gravitation nonlinearity we have shown that the gravitation field of spherically symmetric mass can lead to changes in the gravitational coefficient G.
Measurement of picometre non-linearity in an optical grating encoder using x-ray interferometry
Yacoot, Andrew; Cross, Nigel
2003-01-01
X-ray interferometry has been used to characterize the non-linearity in an optical encoder displacement measuring system. Traceable measurements of the non-linearity have been made and an estimation of the uncertainty associated with the measurements is given. Cyclic errors with a magnitude of up to 50 pm and periodicity of the encoder system (128 nm) have been recorded.
Dual-polarization nonlinear Fourier transform-based optical communication system
DEFF Research Database (Denmark)
Gaiarin, Simone; Perego, A. M.; da Silva, Edson Porto
2018-01-01
communication could potentially overcome these limitations. It relies on a mathematical technique called “nonlinear Fourier transform (NFT)” to exploit the “hidden” linearity of the nonlinear Schrödinger equation as the master model for signal propagation in an optical fiber. We present here the theoretical...
Explicit formulation of second and third order optical nonlinearity in the FDTD framework
Varin, Charles; Emms, Rhys; Bart, Graeme; Fennel, Thomas; Brabec, Thomas
2018-01-01
The finite-difference time-domain (FDTD) method is a flexible and powerful technique for rigorously solving Maxwell's equations. However, three-dimensional optical nonlinearity in current commercial and research FDTD softwares requires solving iteratively an implicit form of Maxwell's equations over the entire numerical space and at each time step. Reaching numerical convergence demands significant computational resources and practical implementation often requires major modifications to the core FDTD engine. In this paper, we present an explicit method to include second and third order optical nonlinearity in the FDTD framework based on a nonlinear generalization of the Lorentz dispersion model. A formal derivation of the nonlinear Lorentz dispersion equation is equally provided, starting from the quantum mechanical equations describing nonlinear optics in the two-level approximation. With the proposed approach, numerical integration of optical nonlinearity and dispersion in FDTD is intuitive, transparent, and fully explicit. A strong-field formulation is also proposed, which opens an interesting avenue for FDTD-based modelling of the extreme nonlinear optics phenomena involved in laser filamentation and femtosecond micromachining of dielectrics.
Third-order optical nonlinearity of N-doped graphene oxide nanocomposites at different GO ratios
Kimiagar, Salimeh; Abrinaei, Fahimeh
2018-05-01
In the present work, the influence of GO ratios on the structural, linear and nonlinear optical properties of nitrogen-doped graphene oxide nanocomposites (N-GO NCs) has been studied. N-GO NCs were synthesized by hydrothermal method. The XRD, FTIR, SEM, and TEM results confirmed the reduction of GO by nitrogen doping. The energy band gaps of N-GO NCs calculated from UV-Vis analyzed by using Tauc plot. To obtain further insight into potential optical changes in the N-GO NCs by increasing GO contents, Z-scan analysis was performed with nanosecond Nd-YAG laser at 532 nm. The nonlinear absorption coefficient, β, and nonlinear refractive index, n2, for N-GO NCs at the laser intensity of 113 MW/cm were measured and an increase was observed in both parameters after addition of nitrogen to GO. The third-order nonlinear optical susceptibilities of N-GO NCs were measured in the order of 10-9 esu. The results showed that N-GO NCs have negative nonlinearity which can be controlled by GO contents to obtain the highest values for nonlinear optical parameters. The nonlinear optical results not only imply that N-GO NCs can serve as an important material in the advancing of optoelectronics but also open new possibilities for the design of new graphene-based materials by variation of N and GO ratios as well as manufacturing conditions.
Latour , Gaël; Echard , Jean-Philippe; Didier , Marie; Schanne-Klein , Marie-Claire
2012-01-01
International audience; We demonstrate multimodal nonlinear optical imaging of historical artifacts by combining Second Harmonic Generation (SHG) and Two-Photon Excited Fluorescence (2PEF) microscopies. We first identify the nonlinear optical response of materials commonly encountered in coatings of cultural heritage artifacts by analyzing one- and multi-layered model samples. We observe 2PEF signals from cochineal lake and sandarac and show that pigments and varnish films can be discriminate...
Energy Technology Data Exchange (ETDEWEB)
Guryev, I. V., E-mail: guryev@ieee.org; Sukhoivanov, I. A., E-mail: guryev@ieee.org; Andrade Lucio, J. A., E-mail: guryev@ieee.org; Manzano, O. Ibarra, E-mail: guryev@ieee.org; Rodriguez, E. Vargaz, E-mail: guryev@ieee.org; Gonzales, D. Claudio, E-mail: guryev@ieee.org; Chavez, R. I. Mata, E-mail: guryev@ieee.org; Gurieva, N. S., E-mail: guryev@ieee.org [University of Guanajuato, Engineering division (Mexico)
2014-05-15
In our work, we investigated the wideband optical filter on the basis of nonlinear photonic crystal. The all-optical flip-flop using ultra-short pulses with duration lower than 200 fs is obtained in such filters. Here we pay special attention to the stability problem of the nonlinear element. To investigate this problem, the temporal response demonstrating the flip-flop have been computed within the certain range of the wavelengths as well as at different input power.
An ultra-efficient nonlinear planar integrated platform for optical signal processing and generation
DEFF Research Database (Denmark)
Pu, Minhao; Ottaviano, Luisa; Semenova, Elizaveta
2017-01-01
This paper will discuss the recently developed integrated platform: AlGaAs-oninsulator and its broad range of nonlinear applications. Recent demonstrations of broadband optical signal processing and efficient frequency comb generations in this platform will be reviewed.......This paper will discuss the recently developed integrated platform: AlGaAs-oninsulator and its broad range of nonlinear applications. Recent demonstrations of broadband optical signal processing and efficient frequency comb generations in this platform will be reviewed....
Nonlinear interactions of focused resonance cone fields with plasmas
International Nuclear Information System (INIS)
Stenzel, R.L.; Gekelman, W.
1977-01-01
A simple yet novel rf exciter structure has been developed for generating remotely intense rf fields in a magnetoplasma. It is a circular line source of radius R in a plane perpendicularB 0 driven with an rf signal at ω 0 E/sub rf/ 2 /nkT/sub e/>0.2, a strong density depression in the focal region (deltan/n>40%) is observed. The density perturbation modifies the cone angle and field distribution. This nonlinear interaction leads to a rapid growth of ion acoustic wave turbulence and a corresponding random rf field distribution in a broadened focal region. The development of the interaction is mapped in space and time
Gradiometer Based on Nonlinear Magneto-Optic Rotation, Phase I
National Aeronautics and Space Administration — This Phase I SBIR project will demonstrate sensitive measurements of magnetic field gradients by nonlinear atomic spectroscopy. The gradients are determined by...
A non-linear theory of strong interactions
International Nuclear Information System (INIS)
Skyrme, T.H.R.
1994-01-01
A non-linear theory of mesons, nucleons and hyperons is proposed. The three independent fields of the usual symmetrical pseudo-scalar pion field are replaced by the three directions of a four-component field vector of constant length, conceived in an Euclidean four-dimensional isotopic spin space. This length provides the universal scaling factor, all other constants being dimensionless; the mass of the meson field is generated by a φ 4 term; this destroys the continuous rotation group in the iso-space, leaving a 'cubic' symmetry group. Classification of states by this group introduces quantum numbers corresponding to isotopic spin and to 'strangeness'; one consequences is that, at least in elementary interactions, charge is only conserved module 4. Furthermore, particle states have not a well-defined parity, but parity is effectively conserved for meson-nucleon interactions. A simplified model, using only two dimensions of space and iso-space, is considered further; the non-linear meson field has solutions with particle character, and an indication is given of the way in which the particle field variables might be introduced as collective co-ordinates describing the dynamics of these particular solutions of the meson field equations, suggesting a unified theory based on the meson field alone. (author). 7 refs
Nonlinear optics for the study of human scar tissue
Ferro, D. P.; Vieira-Damiani, G.; Adam, R. L.; Cesar, C. L.; Metze, Konradin
2012-03-01
Collagen fibers are an essential component of the dynamic process of scarring, which accompanies various diseases. Scar tissue may reveal different morphologic expressions, such as hypertrophic scars or keloids. Collagen fibers can be visualized by fluorescent light when stained with eosin. Second Harmonic Generation (SHG) creates a non linear signal that occurs only in molecules without inversion symmetry and is particularly strong in the collagen fibers arranged in triple helices. The aim of this study was to describe the methodology for the analysis of the density and texture of collagen in keloids, hypertrophic scars and conventional scars. Samples were examined in the National Institute of Science and Technology on Photonics Applied to Cell Biology (INFABIC) at the State University of Campinas. The images were acquired in a multiphoton microscopy LSM 780-NLO Zeiss 40X. Both signals, two-photon fluorescence (TPEF) and SHG, were excited by a Mai-Tai Ti:Sapphire laser at 940 nm. We used a LP490/SP485 NDD filter for SHG, and a BP565-610 NDD filter for fluorescence In each case, ten images were acquired serially (512×512 μm) in Z-stack and joined together to one patchwork-image . Image analysis was performed by a gliding-box-system with in-house made software. Keloids, hypertrophic scars and normal scar tissue show different collagen architecture. Inside an individual case differences of the scar process may be found between central and peripheral parts. In summary, the use of nonlinear optics is a helpful tool for the study of scars tissue.
Relative permittivity in the electrical double layer from nonlinear optics
Boamah, Mavis D.; Ohno, Paul E.; Geiger, Franz M.; Eisenthal, Kenneth B.
2018-06-01
Second harmonic generation (SHG) spectroscopy has been applied to probe the fused silica/water interface at pH 7 and the uncharged 11 ¯ 02 sapphire/water interface at pH 5.2 in contact with aqueous solutions of NaCl, NaBr, NaI, KCl, RbCl, and CsCl as low as several 10 μM. For ionic strengths up to about 0.1 mM, the SHG responses were observed to increase, reversibly for all salts surveyed, when compared to the condition of zero salt added. Further increases in the salt concentration led to monotonic decreases in the SHG response. The SHG increases followed by decreases are found to be consistent with recent reports of phase interference and phase matching in nonlinear optics. By varying the relative permittivity employed in common mean field theories used to describe electrical double layers and by comparing our results to available literature data, we find that models recapitulating the experimental observations are the ones in which (1) the relative permittivity of the diffuse layer is that of bulk water, with other possible values as low as 30, (2) the surface charge density varies with salt concentration, and (3) the charge in the Stern layer or its thickness varies with salt concentration. We also note that the experimental data exhibit sensitivity depending on whether the salt concentration is increased from low to high values or decreased from high to low values, which, however, is not borne out in the fits, at least within the current uncertainties associated with the model point estimates.
Directory of Open Access Journals (Sweden)
Hideki Gotoh
2014-10-01
Full Text Available Optical nonlinear effects are examined using a two-color micro-photoluminescence (micro-PL method in a coherently coupled exciton-biexciton system in a single quantum dot (QD. PL and photoluminescence excitation spectroscopy (PLE are employed to measure the absorption spectra of the exciton and biexciton states. PLE for Stokes and anti-Stokes PL enables us to clarify the nonlinear optical absorption properties in the lowest exciton and biexciton states. The nonlinear absorption spectra for excitons exhibit asymmetric shapes with peak and dip structures, and provide a distinct contrast to the symmetric dip structures of conventional nonlinear spectra. Theoretical analyses with a density matrix method indicate that the nonlinear spectra are caused not by a simple coherent interaction between the exciton and biexciton states but by coupling effects among exciton, biexciton and continuum states. These results indicate that Fano quantum interference effects appear in exciton-biexciton systems at QDs and offer important insights into their physics.
Third-order nonlinear optical response of Ag-CdSe/PVA hybrid nanocomposite
Energy Technology Data Exchange (ETDEWEB)
Tripathi, S.K.; Kaur, Ramneek; Kaur, Jaspreet; Sharma, Mamta [Panjab University, Department of Physics, Center of Advanced Study in Physics, Chandigarh (India)
2015-09-15
Hybrid nanocomposites of II-VI semiconductor nanoparticles are gaining great interest in nonlinear optoelectronic devices. Present work includes the characterization of CdSe polymer nanocomposite prepared by chemical in situ technique. From X-ray diffraction, the hexagonal wurtzite structure of nanoparticles has been confirmed with spherical morphology from transmission electron microscopy. Ag-CdSe hybrid polymer nanocomposite has been prepared chemically at different Ag concentrations. The presence of Ag in hybrid nanocomposite has been confirmed with energy-dispersive X-ray spectroscopy. The effect of varying Ag concentration on the linear and nonlinear optical properties of the nanocomposites has been studied. In linear optical parameters, the linear absorption coefficient, refractive index, extinction coefficient and optical conductivity have been calculated. The third-order nonlinear optical properties have been observed with open- and closed-aperture Z-scan technique. The large nonlinear refractive index ∝10{sup -5} cm{sup 2}/W with self-focusing behaviour is due to the combined effect of quantum confinement and thermo-optical effects. The enhanced nonlinearity with increasing Ag content is due to the surface plasmon resonance, which enhances the local electric field near the nanoparticle surface. Thus, Ag-CdSe hybrid polymer nanocomposite has favourable nonlinear optical properties for various optoelectronic applications. (orig.)
Third-order nonlinear optical response of Ag-CdSe/PVA hybrid nanocomposite
International Nuclear Information System (INIS)
Tripathi, S.K.; Kaur, Ramneek; Kaur, Jaspreet; Sharma, Mamta
2015-01-01
Hybrid nanocomposites of II-VI semiconductor nanoparticles are gaining great interest in nonlinear optoelectronic devices. Present work includes the characterization of CdSe polymer nanocomposite prepared by chemical in situ technique. From X-ray diffraction, the hexagonal wurtzite structure of nanoparticles has been confirmed with spherical morphology from transmission electron microscopy. Ag-CdSe hybrid polymer nanocomposite has been prepared chemically at different Ag concentrations. The presence of Ag in hybrid nanocomposite has been confirmed with energy-dispersive X-ray spectroscopy. The effect of varying Ag concentration on the linear and nonlinear optical properties of the nanocomposites has been studied. In linear optical parameters, the linear absorption coefficient, refractive index, extinction coefficient and optical conductivity have been calculated. The third-order nonlinear optical properties have been observed with open- and closed-aperture Z-scan technique. The large nonlinear refractive index ∝10 -5 cm 2 /W with self-focusing behaviour is due to the combined effect of quantum confinement and thermo-optical effects. The enhanced nonlinearity with increasing Ag content is due to the surface plasmon resonance, which enhances the local electric field near the nanoparticle surface. Thus, Ag-CdSe hybrid polymer nanocomposite has favourable nonlinear optical properties for various optoelectronic applications. (orig.)
Tajaldini, Mehdi; Jafri, Mohd Zubir Mat
2015-04-01
The theory of Nonlinear Modal Propagation Analysis Method (NMPA) have shown significant features of nonlinear multimode interference (MMI) coupler with compact dimension and when launched near the threshold of nonlinearity. Moreover, NMPA have the potential to allow studying the nonlinear MMI based the modal interference to explorer the phenomenon that what happen due to the natural of multimode region. Proposal of all-optical switch based NMPA has approved its capability to achieving the all-optical gates. All-optical gates have attracted increasing attention due to their practical utility in all-optical signal processing networks and systems. Nonlinear multimode interference devices could apply as universal all-optical gates due to significant features that NMPA introduce them. In this Paper, we present a novel Ultra-compact MMI coupler based on NMPA method in low intensity compared to last reports either as a novel design method and potential application for optical NAND, NOR as universal gates on single structure for Boolean logic signal processing devices and optimize their application via studding the contrast ratio between ON and OFF as a function of output width. We have applied NMPA for several applications so that the miniaturization in low nonlinear intensities is their main purpose.
Surface plasmon enhanced third-order optical nonlinearity of Ag nanocomposite film
Energy Technology Data Exchange (ETDEWEB)
Singh, Vijender [Department of Applied Science, N.C. College of Engineering, Israna, Panipat 132107, Haryana (India); Aghamkar, Praveen, E-mail: p-aghamkar@yahoo.in [Department of Physics, Chaudhary Devi Lal University, Sirsa 125055, Haryana (India)
2014-03-17
We obtain a large third-order optical nonlinearity (χ{sup (3)} ≈ 10{sup −10}esu) of silver nanoparticles dispersed in polyvinyl alcohol/tetraethyl orthosilicate matrix using single beam z-scan technique at 532 nm by Q-switched Nd:YAG laser. We have shown that mechanisms responsible for third-order optical nonlinearity of Ag nanocomposite film are reverse saturable absorption (RSA) and self-defocusing in the purlieu of surface plasmon resonance (SPR). Optical band-gap and width of SPR band of Ag nanocomposite film decrease with increasing silver concentration, which leads to enhancement of local electric field and hence third-order optical nonlinearity. Optical limiting, due to RSA has also been demonstrated at 532 nm.
Surface plasmon enhanced third-order optical nonlinearity of Ag nanocomposite film
International Nuclear Information System (INIS)
Singh, Vijender; Aghamkar, Praveen
2014-01-01
We obtain a large third-order optical nonlinearity (χ (3) ≈ 10 −10 esu) of silver nanoparticles dispersed in polyvinyl alcohol/tetraethyl orthosilicate matrix using single beam z-scan technique at 532 nm by Q-switched Nd:YAG laser. We have shown that mechanisms responsible for third-order optical nonlinearity of Ag nanocomposite film are reverse saturable absorption (RSA) and self-defocusing in the purlieu of surface plasmon resonance (SPR). Optical band-gap and width of SPR band of Ag nanocomposite film decrease with increasing silver concentration, which leads to enhancement of local electric field and hence third-order optical nonlinearity. Optical limiting, due to RSA has also been demonstrated at 532 nm
International Nuclear Information System (INIS)
Wu Qingjie; Guo Kangxian; Liu Guanghui; Wu Jinghe
2013-01-01
Polaron effects on the linear and the nonlinear optical absorption coefficients and refractive index changes in cylindrical quantum dots with the radial parabolic potential and the z-direction linear potential with applied magnetic field are theoretically investigated. The optical absorption coefficients and refractive index changes are presented by using the compact-density-matrix approach and iterative method. Numerical calculations are presented for GaAs/AlGaAs. It is found that taking into account the electron-LO-phonon interaction, not only are the linear, the nonlinear and the total optical absorption coefficients and refractive index changes enhanced, but also the total optical absorption coefficients are more sensitive to the incident optical intensity. It is also found that no matter whether the electron-LO-phonon interaction is considered or not, the absorption coefficients and refractive index changes above are strongly dependent on the radial frequency, the magnetic field and the linear potential coefficient.
Choi, Youngsun; Hahn, Choloong; Yoon, Jae Woong; Song, Seok Ho; Berini, Pierre
2017-01-20
Time-asymmetric state-evolution properties while encircling an exceptional point are presently of great interest in search of new principles for controlling atomic and optical systems. Here, we show that encircling-an-exceptional-point interactions that are essentially reciprocal in the linear interaction regime make a plausible nonlinear integrated optical device architecture highly nonreciprocal over an extremely broad spectrum. In the proposed strategy, we describe an experimentally realizable coupled-waveguide structure that supports an encircling-an-exceptional-point parametric evolution under the influence of a gain saturation nonlinearity. Using an intuitive time-dependent Hamiltonian and rigorous numerical computations, we demonstrate strictly nonreciprocal optical transmission with a forward-to-backward transmission ratio exceeding 10 dB and high forward transmission efficiency (∼100%) persisting over an extremely broad bandwidth approaching 100 THz. This predicted performance strongly encourages experimental realization of the proposed concept to establish a practical on-chip optical nonreciprocal element for ultra-short laser pulses and broadband high-density optical signal processing.
International Nuclear Information System (INIS)
Torres-Torres, C.; García-Cruz, M.L.; Castañeda, L.; Rangel Rojo, R.; Tamayo-Rivera, L.; Maldonado, A.; Avendaño-Alejo, M.
2012-01-01
Chromium doped zinc oxide thin solid films were deposited on soda–lime glass substrates. The photoconductivity of the material and its influence on the optical behavior was evaluated. A non-alkoxide sol–gel synthesis approach was used for the preparation of the samples. An enhancement of the photoluminescence response exhibited by the resulting photoconductive films with embedded chromium nanoclusters is presented. The modification in the photoconduction induced by a 445 nm wavelength was measured and then associated with the participation of the optical absorptive response. In order to investigate the third order optical nonlinearities of the samples, a standard time-resolved Optical Kerr Gate configuration with 80 fs pulses at 830 nm was used and a quasi-instantaneous pure electronic nonlinearity without the contribution of nonlinear optical absorption was observed. We estimate that from the inclusion of Cr nanoclusters into the sample results a strong optical Kerr effect originated by quantum confinement. The large photoluminescence response and the important refractive nonlinearity of the photoconductive samples seem to promise potential applications for the development of multifunctional all-optical nanodevices. - Highlights: ► Enhancement in photoluminescence for chromium doped zinc oxide films is presented. ► A strong and ultrafast optical Kerr effect seems to result from quantum confinement. ► Photoconductive properties for optical and optoelectronic functions were observed.
Energy Technology Data Exchange (ETDEWEB)
Torres-Torres, C., E-mail: crstorres@yahoo.com.mx [Seccion de Estudios de Posgrado e Investigacion, ESIME-Z, Instituto Politecnico Nacional, Mexico, DF 07738 (Mexico); Garcia-Cruz, M.L. [Centro de Investigacion en Dispositivos Semiconductores, Benemerita Universidad Autonoma de Puebla, A. P. J-48, Puebla 72570, Mexico (Mexico); Castaneda, L., E-mail: luisca@sirio.ifuap.buap.mx [Instituto de Fisica, Benemerita Universidad Autonoma de Puebla, A. P. J-48, Puebla 72570, Mexico (Mexico); Rangel Rojo, R. [CICESE/Depto. de Optica, A. P. 360, Ensenada, BC 22860 (Mexico); Tamayo-Rivera, L. [Instituto de Fisica, Universidad Nacional Autonoma de Mexico, Mexico, DF 01000 (Mexico); Maldonado, A. [Depto. de Ing. Electrica, CINVESTAV IPN-SEES, A. P. 14740, Mexico DF 07000 (Mexico); Avendano-Alejo, M., E-mail: imax_aa@yahoo.com.mx [Centro de Ciencias Aplicadas y Desarrollo Tecnologico, Universidad Nacional Autonoma de Mexico, A. P. 70-186, 04510, DF (Mexico); and others
2012-04-15
Chromium doped zinc oxide thin solid films were deposited on soda-lime glass substrates. The photoconductivity of the material and its influence on the optical behavior was evaluated. A non-alkoxide sol-gel synthesis approach was used for the preparation of the samples. An enhancement of the photoluminescence response exhibited by the resulting photoconductive films with embedded chromium nanoclusters is presented. The modification in the photoconduction induced by a 445 nm wavelength was measured and then associated with the participation of the optical absorptive response. In order to investigate the third order optical nonlinearities of the samples, a standard time-resolved Optical Kerr Gate configuration with 80 fs pulses at 830 nm was used and a quasi-instantaneous pure electronic nonlinearity without the contribution of nonlinear optical absorption was observed. We estimate that from the inclusion of Cr nanoclusters into the sample results a strong optical Kerr effect originated by quantum confinement. The large photoluminescence response and the important refractive nonlinearity of the photoconductive samples seem to promise potential applications for the development of multifunctional all-optical nanodevices. - Highlights: Black-Right-Pointing-Pointer Enhancement in photoluminescence for chromium doped zinc oxide films is presented. Black-Right-Pointing-Pointer A strong and ultrafast optical Kerr effect seems to result from quantum confinement. Black-Right-Pointing-Pointer Photoconductive properties for optical and optoelectronic functions were observed.
Nonlinear Pulse Shaping in Fibres for Pulse Generation and Optical Processing
Directory of Open Access Journals (Sweden)
Sonia Boscolo
2012-01-01
Full Text Available The development of new all-optical technologies for data processing and signal manipulation is a field of growing importance with a strong potential for numerous applications in diverse areas of modern science. Nonlinear phenomena occurring in optical fibres have many attractive features and great, but not yet fully explored, potential in signal processing. Here, we review recent progress on the use of fibre nonlinearities for the generation and shaping of optical pulses and on the applications of advanced pulse shapes in all-optical signal processing. Amongst other topics, we will discuss ultrahigh repetition rate pulse sources, the generation of parabolic shaped pulses in active and passive fibres, the generation of pulses with triangular temporal profiles, and coherent supercontinuum sources. The signal processing applications will span optical regeneration, linear distortion compensation, optical decision at the receiver in optical communication systems, spectral and temporal signal doubling, and frequency conversion.
International Nuclear Information System (INIS)
Konar, S.; Mishra, Manoj; Jana, S.
2006-01-01
The role of quintic nonlinearity on the propagation characteristics of optical solitons in dispersion managed optical communication systems has been presented in this paper. It has been shown that quintic nonlinearity has only marginal influence on single pulse propagation. However, numerical simulation has been undertaken to reveal that quintic nonlinearity reduces collision distance between neighbouring pulses of the same channel. It is found that for lower map strength the collapse distance between intra channel pulses is very much sensitive to the dispersion map strength
Experimental investigations of optical nonlinearities in semiconductor-doped glass waveguides
International Nuclear Information System (INIS)
Dannberg, P.; Possner, T.; Braeuer, A.; Bartuch, U.
1988-01-01
Both, thermal and electronic optical nonlinearities are studied in semiconductor-doped glass (SDG) waveguides which are fabricated in commercially available sharp-cut filters by Cs + -K + ion exchange. The relaxation time in photodarkened substrates is measured to be 30 ps. By means of a prism coupling set-up the saturation value of the nonlinear index change is determined. Furthermore, a high stability dual-beam interferometer is presented for the measurement of both, thermal and electronic nonlinear refractive index n 2 in planar waveguides. Conclusions about the application of SDG to opto-optical switching are given. (author)
An, Honglin; Fleming, Simon
2005-05-02
The spatial distribution of second-order nonlinearity in thermally poled optical fibers was characterized by second-harmonic microscopy. The second-order nonlinearity was found to be confined to a thin layer close to the anode surface and progressed further into the silica as the poling time increased. Position uncertainty of the anode metal wire was observed to have an effect, as the nonlinear layers were found not always symmetrically located around the nearest points between the anode and cathode. Optical microscopy results were obtained on etched poled fiber cross-sections and compared with those from second-harmonic microscopy.
Light-induced second-order nonlinear optical properties of molecular materials
International Nuclear Information System (INIS)
Fiorini, Celine
1995-01-01
We present a theoretical and experimental study of all-optical orientation. The work focusses more particularly on the realization of poled polymers for quadratic nonlinear optics. It is shown that the coherent superposition of two beams at fundamental and second harmonic frequencies results in the breaking of the former centro-symmetry of the material. The source is a Neodymium-YAG laser delivering 25 ps pulses at 1064 nm. The incident second-harmonic beam is obtained by frequency doubling in a KDP crystal. Using a phase conjugation configuration based on six-wave mixing interactions, we have Investigated in detail the mechanism of photo-induced second-harmonic generation in initially centrosymmetric materials. It is shown that the light-induced non-centro-symmetry is due to an orientational hole burning of the molecules. The process involves interference effects between one and two photon absorptions. Experiments are performed in various solutions of an azo-dye molecule (Disperse Red One). The possibility of inducing quasi-permanent second-order susceptibility in a PMMA polymer matrix doped with the azo-dye molecule of Disperse Red One is also demonstrated. The method of all-optical poling consists in a seeding type process with alternate writing and probing phases. Permanent orientation of the molecules can be described in terms of photo-isomerization processes. It leads to a poling of the molecules with a spatial modulation which is phase-matched for frequency doubling. Relevant parameters leading to an efficient polarisation of the sample are identified. A theoretical modelling of the different phenomena observed is proposed. Last part of the study is devoted to an enlarged study of the potentialities offered by this dual-frequency holography technique: orientation of octupolar molecules, polarisation of highly transparent materials. We also show that the new techniques developed during this work can also reveal to be complementary methods for nonlinear
Wang, Chun-Chin; Li, Feng-Chieh; Lin, Sung-Jan; Lo, Wen; Dong, Chen-Yuan
2007-07-01
In this investigation, we used in vivo nonlinear optical microscopy to image normal and carcinogen DMBA treated skin tissues of nude mice. We acquired two-photon autofluroescence and second harmonic generation (SHG) images of the skin tissue, and applied the ASI (Autofluorescence versus SHG Index) to the resulting image. This allows us to visualize and quantify the interaction between mouse skin cells and the surrounding connective tissue. We found that as the imaging depth increases, ASI has a different distribution in the normal and the treated skin tissues. Since the DMBA treated skin eventually became squamous cell carcinoma (SCC), our results show that the physiological changes to mouse skin en route to become cancer can be effectively tracked by multiphoton microscopy. We envision this approach to be effective in studying tumor biology and tumor treatment procedures.
1991-03-13
combination50 with a dynamic grating diffraction modelO . Considering o 0 a polarlsatlon grating on a homoetropic aligned nematlc ’-i 40 filmi the optical...nonlinearities of solutions of chloroaluminumphthalocyanine (CAP) in methanol and a silicon naphthalocyanine (Nc) derivative, SiNc( OSi (hexyl)3)2 or
Nonlinear optical diagnostic of semimagnetic semiconductors Pb1-xYb xX (X = S, Se, Te)
International Nuclear Information System (INIS)
Nouneh, K.; Kityk, I.V.; Viennois, R.; Benet, S.; Charar, S.; Plucinski, K.J.
2007-01-01
Nonlinear optical measurements were performed to elucidate the influence of magnetic ions on the behavior of charge carriers in magnetic semiconductors-Pb 1-x Yb x X (X = S, Se, Te at x = 1-3%). It was shown that nonlinear optical methods could be used as sensitive tools for investigations of electron-phonon anharmonicity near low-temperature semiconductor-insulator phase transitions. There exists a difference between surface and bulk-like contributions to the nonlinear optical effects. It was shown that only low-temperature Two Photon Absorption (TPA) oscillator may be related to the number of the electron-phonon anharmonic modes responsible for the observed phase transformation. The explanation of the anomalous temperature dependences is given in accordance with dipole momentum's behaviors determined by low-temperature spin-spin interactions and by electron-phonon anharmonic interactions. We have discovered that low-temperature dependence of specific heat of Pb 1-x R x Te (R = Yb, Pr with x = 3% and 1.6%, respectively) exhibits a non-magnetic order caused by large electron-phonon contributions and structural disorder effects
Nonlinear dynamic soil-structure interaction in earthquake engineering
International Nuclear Information System (INIS)
Nieto-Ferro, Alex
2013-01-01
The present work addresses a computational methodology to solve dynamic problems coupling time and Laplace domain discretizations within a domain decomposition approach. In particular, the proposed methodology aims at meeting the industrial need of performing more accurate seismic risk assessments by accounting for three-dimensional dynamic soil-structure interaction (DSSI) in nonlinear analysis. Two subdomains are considered in this problem. On the one hand, the linear and unbounded domain of soil which is modelled by an impedance operator computed in the Laplace domain using a Boundary Element (BE) method; and, on the other hand, the superstructure which refers not only to the structure and its foundations but also to a region of soil that possibly exhibits nonlinear behaviour. The latter sub-domain is formulated in the time domain and discretized using a Finite Element (FE) method. In this framework, the DSSI forces are expressed as a time convolution integral whose kernel is the inverse Laplace transform of the soil impedance matrix. In order to evaluate this convolution in the time domain by means of the soil impedance matrix (available in the Laplace domain), a Convolution Quadrature-based approach called the Hybrid Laplace-Time domain Approach (HLTA), is thus introduced. Its numerical stability when coupled to Newmark time integration schemes is subsequently investigated through several numerical examples of DSSI applications in linear and nonlinear analyses. The HLTA is finally tested on a more complex numerical model, closer to that of an industrial seismic application, and good results are obtained when compared to the reference solutions. (author)
Optical nonlinearities of excitonic states in atomically thin 2D transition metal dichalcogenides
Energy Technology Data Exchange (ETDEWEB)
Soh, Daniel Beom Soo [Sandia National Lab. (SNL-CA), Livermore, CA (United States). Proliferation Signatures Discovery and Exploitation Department
2017-08-01
We calculated the optical nonlinearities of the atomically thin monolayer transition metal dichalcogenide material (particularly MoS_{2}), particularly for those linear and nonlinear transition processes that utilize the bound exciton states. We adopted the bound and the unbound exciton states as the basis for the Hilbert space, and derived all the dynamical density matrices that provides the induced current density, from which the nonlinear susceptibilities can be drawn order-by-order via perturbative calculations. We provide the nonlinear susceptibilities for the linear, the second-harmonic, the third-harmonic, and the kerr-type two-photon processes.
Girardeau, Vadim; Goloni, Carolina; Jacquin, Olivier; Hugon, Olivier; Inglebert, Mehdi; Lacot, Eric
2016-12-01
In this article, we study the nonlinear dynamics of a laser subjected to frequency shifted optical reinjection coming back from a vibrating target. More specifically, we study the nonlinear dynamical coupling between the carrier and the vibration signal. The present work shows how the nonlinear amplification of the vibration spectrum is related to the strength of the carrier and how it must be compensated to obtain accurate (i.e., without bias) vibration measurements. The theoretical predictions, confirmed by numerical simulations, are in good agreement with the experimental data. The main motivation of this study is the understanding of the nonlinear response of a laser optical feedback imaging sensor for quantitative phase measurements of small vibrations in the case of strong optical feedback.
Theoretical investigation of intensity-dependent optical nonlinearity in graphene-aided D-microfiber
Shah, Manoj Kumar; Lu, Rongguo; Zhang, Yali; Ye, Shengwei; Zhang, Shangjian; Liu, Yong
2018-01-01
We theoretically investigate the intensity-dependent optical nonlinearity in graphene-aided D-microfiber, by tuning the chemical potential of graphene and varying radial distance and radii of the D-microfiber. Utilizing an interplay between graphene and the enhanced evanescent field of a guided mode in the waveguide of interest, the net utility of nonlinear coefficient is harnessed up to a very high value of 106 W-1m-1. Importantly, which is ∼ two orders of magnitude larger than in PMMA-graphene-PMMA waveguide. The highly dispersive nature of the waveguide, D ∼ 103 ps/nm-km, and large nonlinear figure-of-merit, FOMNL ∼ 1.29, have raised the possibilities of utilizing slow light structures to operate devices at few watts power level with microscale length. These studies have opened one window towards the next-generation all fiber-optic graphene nonlinear optical devices.
International Nuclear Information System (INIS)
Tian Bo; Gao Yitian
2005-01-01
A realistic, inhomogeneous fiber in the optical communication systems can be described by the perturbed nonlinear Schrodinger model (also named as the normalized nonlinear Schrodinger model with periodically varying coefficients, dispersion managed nonlinear Schrodinger model or nonlinear Schrodinger model with variable coefficients). Hereby, we extend to this model a direct method, perform symbolic computation and obtain two families of the exact, analytic bright-solitonic solutions, with or without the chirp respectively. The parameters addressed include the shape of the bright soliton, soliton amplitude, inverse width of the soliton, chirp, frequency, center of the soliton and center of the phase of the soliton. Of optical and physical interests, we discuss some previously-published special cases of our solutions. Those solutions could help the future studies on the optical communication systems. ms
Theoretical studies of some nonlinear laser-plasma interactions
International Nuclear Information System (INIS)
Cohen, B.I.
1975-01-01
The nonlinear coupling of intense, monochromatic, electromagnetic radiation with plasma is considered in a number of special cases. The first part of the thesis serves as an introduction to three-wave interactions. A general formulation of the stimulated scattering of transverse waves by longitudinal modes in a warm, unmagnetized, uniform plasma is constructed. A general dispersion relation is derived that describes Raman and Brillouin scattering, modulational instability, and induced Thomson scattering. Raman scattering (the scattering of a photon into another photon and an electron plasma wave) is investigated as a possible plasma heating scheme. Analytic theory complemented by computer simulation is presented describing the nonlinear mode coupling of laser light with small and large amplitude, resonantly excited electron plasma waves. The simulated scattering of a coherent electromagnetic wave by low frequency density perturbations in homogeneous plasma is discussed. A composite picture of the linear dispersion relations for filamentation and Brillouin scattering is constructed. The absolute instability of Brillouin weak and strong coupling by analytic and numerical means is described
Asymptotic approach for the nonlinear equatorial long wave interactions
International Nuclear Information System (INIS)
Ramirez Gutierrez, Enver; Silva Dias, Pedro L; Raupp, Carlos
2011-01-01
In the present work we use an asymptotic approach to obtain the long wave equations. The shallow water equation is put as a function of an external parameter that is a measure of both the spatial scales anisotropy and the fast to slow time ratio. The values given to the external parameters are consistent with those computed using typical values of the perturbations in tropical dynamics. Asymptotically, the model converge toward the long wave model. Thus, it is possible to go toward the long wave approximation through intermediate realizable states. With this approach, the resonant nonlinear wave interactions are studied. To simplify, the reduced dynamics of a single resonant triad is used for some selected equatorial trios. It was verified by both theoretical and numerical results that the nonlinear energy exchange period increases smoothly as we move toward the long wave approach. The magnitude of the energy exchanges is also modified, but in this case depends on the particular triad used and also on the initial energy partition among the triad components. Some implications of the results for the tropical dynamics are discussed. In particular, we discuss the implications of the results for El Nino and the Madden-Julian in connection with other scales of time and spatial variability.
Nonlinear Kinetics on Lattices Based on the Kinetic Interaction Principle
Directory of Open Access Journals (Sweden)
Giorgio Kaniadakis
2018-06-01
Full Text Available Master equations define the dynamics that govern the time evolution of various physical processes on lattices. In the continuum limit, master equations lead to Fokker–Planck partial differential equations that represent the dynamics of physical systems in continuous spaces. Over the last few decades, nonlinear Fokker–Planck equations have become very popular in condensed matter physics and in statistical physics. Numerical solutions of these equations require the use of discretization schemes. However, the discrete evolution equation obtained by the discretization of a Fokker–Planck partial differential equation depends on the specific discretization scheme. In general, the discretized form is different from the master equation that has generated the respective Fokker–Planck equation in the continuum limit. Therefore, the knowledge of the master equation associated with a given Fokker–Planck equation is extremely important for the correct numerical integration of the latter, since it provides a unique, physically motivated discretization scheme. This paper shows that the Kinetic Interaction Principle (KIP that governs the particle kinetics of many body systems, introduced in G. Kaniadakis, Physica A 296, 405 (2001, univocally defines a very simple master equation that in the continuum limit yields the nonlinear Fokker–Planck equation in its most general form.
Nonlinear optics at the single-photon level inside a hollow core fiber
DEFF Research Database (Denmark)
Hofferberth, Sebastian; Peyronel, Thibault; Liang, Qiyu
2011-01-01
Cold atoms inside a hollow core fiber provide an unique system for studying optical nonlinearities at the few-photon level. Confinement of both atoms and photons inside the fiber core to a diameter of just a few wavelengths results in high electric field intensity per photon and large optical...
Duan, Y.; Ju, C.G.; Yang, G.; Fron, E.; Coutino-Gonzalez, E.; Semin, S.V.; Fan, C.C.; Balok, R.S.; Cremers, J.; Tinnemans, P.T.; Feng, Y.Q.; Li, Y.L.; Hofkens, J.; Rowan, A.E.; Rasing, T.H.M.; Xu, J.L.
2016-01-01
The discovery of the phenomenon known as aggregation-induced emission (AIE) has opened the door to a variety of brilliant organic solid-state light-emitting materials. While AIE is well established in linear optics, the development of AIE luminogens (AIEgens) with highly efficient nonlinear optical
Gieseking, Rebecca L.
2014-10-16
Polymethine dyes in dilute solutions show many of the electronic and optical properties required for all-optical switching applications. However, in the form of thin films, their aggregation and interactions with counterions do generally strongly limit their utility. Here, we present a theoretical approach combining molecular-dynamics simulations and quantum-chemical calculations to describe the bulk molecular packing of streptocyanines (taken as representative of simple polymethines) with counterions of different hardness (Cl and BPh4 ) and understand the impact on the optical properties. The accuracy of the force field we use is verified by reproducing experimental crystal parameters as well as the configurations of polymethine/counterion complexes obtained from electronic-structure calculations. The aggregation characteristics can be understood in terms of both polymethinecounterion and polymethinepolymethine interactions. The counterions are found to localize near one end of the streptocyanine backbones, and the streptocyanines form a broad range of aggregates with significant electronic couplings between neighboring molecules. As a consequence, the linear and nonlinear optical properties are substantially modified in the bulk. By providing an understanding of the relationship between the molecular interactions and the bulk optical properties, our results point to a clear strategy for designing polymethine and counterion molecular structures and optimizing the materials properties for all-optical switching applications.
Gieseking, Rebecca L.; Mukhopadhyay, Sukrit; Shiring, Stephen B.; Risko, Chad; Bredas, Jean-Luc
2014-01-01
Polymethine dyes in dilute solutions show many of the electronic and optical properties required for all-optical switching applications. However, in the form of thin films, their aggregation and interactions with counterions do generally strongly limit their utility. Here, we present a theoretical approach combining molecular-dynamics simulations and quantum-chemical calculations to describe the bulk molecular packing of streptocyanines (taken as representative of simple polymethines) with counterions of different hardness (Cl and BPh4 ) and understand the impact on the optical properties. The accuracy of the force field we use is verified by reproducing experimental crystal parameters as well as the configurations of polymethine/counterion complexes obtained from electronic-structure calculations. The aggregation characteristics can be understood in terms of both polymethinecounterion and polymethinepolymethine interactions. The counterions are found to localize near one end of the streptocyanine backbones, and the streptocyanines form a broad range of aggregates with significant electronic couplings between neighboring molecules. As a consequence, the linear and nonlinear optical properties are substantially modified in the bulk. By providing an understanding of the relationship between the molecular interactions and the bulk optical properties, our results point to a clear strategy for designing polymethine and counterion molecular structures and optimizing the materials properties for all-optical switching applications.
International Nuclear Information System (INIS)
Lee, P.-F.; Yeh, Alvin T.; Bayless, Kayla J.
2009-01-01
The interactions between endothelial cells (ECs) and the extracellular matrix (ECM) are fundamental in mediating various steps of angiogenesis, including cell adhesion, migration and sprout formation. Here, we used a noninvasive and non-destructive nonlinear optical microscopy (NLOM) technique to optically image endothelial sprouting morphogenesis in three-dimensional (3D) collagen matrices. We simultaneously captured signals from collagen fibers and endothelial cells using second harmonic generation (SHG) and two-photon excited fluorescence (TPF), respectively. Dynamic 3D imaging revealed EC interactions with collagen fibers along with quantifiable alterations in collagen matrix density elicited by EC movement through and morphogenesis within the matrix. Specifically, we observed increased collagen density in the area between bifurcation points of sprouting structures and anisotropic increases in collagen density around the perimeter of lumenal structures, but not advancing sprout tips. Proteinase inhibition studies revealed membrane-associated matrix metalloproteinase were utilized for sprout advancement and lumen expansion. Rho-associated kinase (p160ROCK) inhibition demonstrated that the generation of cell tension increased collagen matrix alterations. This study followed sprouting ECs within a 3D matrix and revealed that the advancing structures recognize and significantly alter their extracellular environment at the periphery of lumens as they progress
Energy Technology Data Exchange (ETDEWEB)
Divya Bharathi, M.; Ahila, G.; Mohana, J. [Department of Physics, Presidency College, Chennai 600005 (India); Chakkaravarthi, G. [Department of Physics, CPCL Polytechnic College, Chennai 600068 (India); Anbalagan, G., E-mail: anbu24663@yahoo.co.in [Department of Nuclear Physics, University of Madras, Chennai 600025 (India)
2017-05-01
A neoteric organic third order nonlinear optical material 8-hydroxyquinolinium 2-chloro-5-nitrobenzoate dihydrate (8HQ2C5N) was grown by slow cooling technique using ethanol: water (1:1) mixed solvent. The calculated low value of average etch pit solidity (4.12 × 10{sup 3} cm{sup −2}) indicated that the title crystal contain less defects. From the single crystal X-ray diffraction data, it was endowed that 8HQ2C5N crystal belongs to the monoclinic system with centrosymmetric space group P2{sub 1}/c and the cell parameters values, a = 9.6546 (4) Ǻ, b = 7.1637(3) Ǻ, c = 24.3606 (12) Ǻ, α = γ = 90°, β = 92.458(2)° and volume = 1683.29(13) Ǻ{sup 3}. The FT-IR and FT-Raman spectrum were used to affirm the functional group of the title compound. The chemical structure of 8HQ2C5N was scrutinized by {sup 13}C and {sup 1}H NMR spectral analysis and thermal stability through the differential scanning calorimetry study. Using optical studies the lower cut-off wavelength and optical band gap of 8HQ2C5N were found to be 364 nm and 3.17 eV respectively. Using the single oscillator model suggested by Wemple – Didomenico, the oscillator energy (E{sub o}), the dispersion energy (E{sub d}) and static dielectric constant (ε{sub o}) were estimated. The third-order susceptibility were determined as Im χ{sup (3)} = 2.51 × 10{sup −5} esu and Re χ{sup (3)} = 4.46 × 10{sup −7} esu. The theoretical third-order nonlinear optical susceptibility χ{sup (3)} was calculated and the results were compared with experimental value. Photoluminescence spectrum of 8HQ2C5N crystal showed the yellow emission. The crystal had the single shot laser damage threshold of 5.562 GW/cm{sup 2}. Microhardness measurement showed that 8HQ2C5N belongs to a soft material category. - Highlights: • A new organic single crystals were grown and the crystal structure was reported. • Crystal possess, good transmittance, thermal and mechanical stability. • Single shot LDT value is found to be
Interaction between two point-like charges in nonlinear electrostatics
Energy Technology Data Exchange (ETDEWEB)
Breev, A.I. [Tomsk State University, Tomsk (Russian Federation); Tomsk Polytechnic University, Tomsk (Russian Federation); Shabad, A.E. [P.N. Lebedev Physical Institute, Moscow (Russian Federation); Tomsk State University, Tomsk (Russian Federation)
2018-01-15
We consider two point-like charges in electrostatic interaction within the framework of a nonlinear model, associated with QED, that provides finiteness of their field energy. We find the common field of the two charges in a dipole-like approximation, where the separation between them R is much smaller than the observation distance r: with the linear accuracy with respect to the ratio R/r, and in the opposite approximation, where R >> r, up to the term quadratic in the ratio r/R. The consideration proposes the law a + bR{sup 1/3} for the energy, when the charges are close to one another, R → 0. This leads to the singularity of the force between them to be R{sup -2/3}, which is weaker than the Coulomb law, R{sup -2}. (orig.)
Interaction between two point-like charges in nonlinear electrostatics
Breev, A. I.; Shabad, A. E.
2018-01-01
We consider two point-like charges in electrostatic interaction within the framework of a nonlinear model, associated with QED, that provides finiteness of their field energy. We find the common field of the two charges in a dipole-like approximation, where the separation between them R is much smaller than the observation distance r : with the linear accuracy with respect to the ratio R / r, and in the opposite approximation, where R≫ r, up to the term quadratic in the ratio r / R. The consideration proposes the law a+b R^{1/3} for the energy, when the charges are close to one another, R→ 0. This leads to the singularity of the force between them to be R^{-2/3}, which is weaker than the Coulomb law, R^{-2}.
Synthesis, characterization and third-order nonlinear optical ...
Indian Academy of Sciences (India)
2016-09-20
Sep 20, 2016 ... the past, several strategies have been evolved to enhance the third-order nonlinear ..... retical fit using the formulation given in ref. [22]. Fit param- ..... Acknowledgement. The corresponding author acknowledges the financial.
International Nuclear Information System (INIS)
Wu, Jinghe; Guo, Kangxian; Liu, Guanghui
2014-01-01
Polaron effects on nonlinear optical rectification in asymmetrical Gaussian potential quantum wells are studied by the effective mass approximation and the perturbation theory. The numerical results show that nonlinear optical rectification coefficients are strongly dependent on the barrier hight V 0 of the Gaussian potential quantum wells, the range L of the confinement potential and the electric field F. Besides, the numerical results show that no matter how V 0 , L and F change, taking into consideration polaron effects, the optical rectification coefficients χ 0 (2) get greatly enhanced.
CW all optical self switching in nonlinear chalcogenide nano plasmonic directional coupler
Motamed-Jahromi, Leila; Hatami, Mohsen
2018-04-01
In this paper we obtain the coupling coefficient of plasmonic directional coupler (PDC) made up of two parallel monolayer waveguides filled with high nonlinear chalcogenide material for TM mode in continues wave (CW) regime. In addition, we assume each waveguides acts as a perturbation to other waveguide. Four nonlinear-coupled equations are derived. Transfer distances are numerically calculated and used for deriving length of all optical switch. The length of designed switch is in the range of 10-1000 μm, and the switching power is in the range of 1-100 W/m. Obtained values are suitable for designing all optical elements in the integrated optical circuits.
Alkali-Responsive Absorption Spectra and Third-Order Optical Nonlinearities of Imino Squaramides
International Nuclear Information System (INIS)
Li Zhong-Yu; Xu Song; Zhou Xin-Yu; Zhang Fu-Shi
2012-01-01
Third-order optical nonlinearities and dynamic responses of two imino squaramides under neutral and base conditions were studied using the femtosecond degenerate four-wave mixing technique at 800 nm. Ultrafast optical responses have been observed and the magnitude of the second-order hyperpolarizabilities of the squaramides has been measured to be as large as 10 −31 esu. The absorption spectra, color of solution, and third-order optical nonlinearities of two imino squaramides change with the addition of sodium hydroxide. The γ value under the base condition for each dye is approximately 1.25 times larger than that under neutral conditions. (fundamental areas of phenomenology(including applications))
Nonlinear optical behaviour of absorbing CdSxSe1-x interference filters
International Nuclear Information System (INIS)
Ferencz, K.; Szipoecs, R.
1988-01-01
First experimental results of nonlinear, thin film interference filter wedges with mixed CdS x Se 1-x as spacer material at the 633 nm wavelength of He-Ne laser are reported. Optical bistability is observed with less than 7.5 mW of optical power in single-cavity structures. The change in refractive index is found to be positive which is in accordance with the thermal mechanism of nonlinearity. Producing a double-cavity structure a device is obtained which works as an optical astable multivibrator having periodical change of transmission as the function of time. (author)
Nonlinear interaction and wave breaking with a submerged porous structure
Hsieh, Chih-Min; Sau, Amalendu; Hwang, Robert R.; Yang, W. C.
2016-12-01
Numerical simulations are performed to investigate interactive velocity, streamline, turbulent kinetic energy, and vorticity perturbations in the near-field of a submerged offshore porous triangular structure, as Stokes waves of different heights pass through. The wave-structure interaction and free-surface breaking for the investigated flow situations are established based on solutions of 2D Reynolds Averaged Navier-Stokes equations in a Cartesian grid in combination with K-ɛ turbulent closure and the volume of fluid methodology. The accuracy and stability of the adopted model are ascertained by extensive comparisons of computed data with the existing experimental and theoretical findings and through efficient predictions of the internal physical kinetics. Simulations unfold "clockwise" and "anticlockwise" rotation of fluid below the trough and the crest of the viscous waves, and the penetrated wave energy creates systematic flow perturbation in the porous body. The interfacial growths of the turbulent kinetic energy and the vorticity appear phenomenal, around the apex of the immersed structure, and enhanced significantly following wave breaking. Different values of porosity parameter and two non-porous cases have been examined in combination with varied incident wave height to reveal/analyze the nonlinear flow behavior in regard to local spectral amplification and phase-plane signatures. The evolution of leading harmonics of the undulating free-surface and the vertical velocity exhibits dominating roles of the first and the second modes in inducing the nonlinearity in the post-breaking near-field that penetrates well below the surface layer. The study further suggests the existence of a critical porosity that can substantially enhance the wave-shoaling and interface breaking.
Evaluation of third order nonlinear optical parameters of CdS/PVA nanocomposite
Energy Technology Data Exchange (ETDEWEB)
Sharma, Mamta [Department of Physics, Center of Advanced Study in Physics, Panjab University, Chandigarh-160014 (India); Department of Applied Sciences (Physics), UIET, Panjab University, Chandigarh-160014 (India); Tripathi, S. K., E-mail: surya@pu.ac.in, E-mail: surya-tr@yahoo.com [Department of Physics, Center of Advanced Study in Physics, Panjab University, Chandigarh-160014 (India)
2015-06-24
CdS nanoparticles dispersed in PVA are prepared by Chemical method at room temperature. The nonlinear optical parameters such as nonlinear absorption (β), nonlinear refractive index (n{sub 2}) and nonlinear susceptibility (χ{sup 3}) are calculated for this sample by using Z-scan technique. CdS/PVA samples show the two photon absorption mechanism. The third order nonlinear susceptibility is calculated from n{sub 2} and β and is found to be of the order of 10{sup −7} – 10{sup −8} m{sup 2}/V{sup 2}. The larger value of third order nonlinear susceptibility is due to dielectric and quantum confinement effect.
Linear and Nonlinear Optical Properties of Micrometer-Scale Gold Nanoplates
International Nuclear Information System (INIS)
Liu Xiao-Lan; Peng Xiao-Niu; Yang Zhong-Jian; Li Min; Zhou Li
2011-01-01
Micrometer-scale gold nanoplates have been synthesized in high yield through a polyol process. The morphology, crystal structure and linear optical extinction of the gold nanoplates have been characterized. These gold nanoplates are single-crystalline with triangular, truncated triangular and hexagonal shapes, exhibiting strong surface plasmon resonance (SPR) extinction in the visible and near-infrared (NIR) region. The linear optical properties of gold nanoplates are also investigated by theoretical calculations. We further investigate the nonlinear optical properties of the gold nanoplates in solution by Z-scan technique. The nonlinear absorption (NLA) coefficient and nonlinear refraction (NLR) index are measured to be 1.18×10 2 cm/GW and −1.04×10 −3 cm 2 /GW, respectively. (condensed matter: electronic structure, electrical, magnetic, and optical properties)
A nonlinear plasmonic resonator for three-state all-optical switching
Amin, Muhammad
2014-01-01
A nonlinear plasmonic resonator design is proposed for three-state all-optical switching at frequencies including near infrared and lower red parts of the spectrum. The tri-stable response required for three-state operation is obtained by enhancing nonlinearities of a Kerr medium through multiple (higher order) plasmons excited on resonator\\'s metallic surfaces. Indeed, simulations demonstrate that exploitation of multiple plasmons equips the proposed resonator with a multi-band tri-stable response, which cannot be obtained using existing nonlinear plasmonic devices that make use of single mode Lorentzian resonances. Multi-band three-state optical switching that can be realized using the proposed resonator has potential applications in optical communications and computing. © 2014 Optical Society of America.
Nonlinear optical measurements of conducting copolymers of aniline under CW laser excitation
Pramodini, S.; Poornesh, P.
2015-08-01
Synthesis and measurements of third-order optical nonlinearity and optical limiting of conducting copolymers of aniline are presented. Single beam z-scan technique was employed for the nonlinear optical studies. Continuous wave He-Ne laser operating at 633 nm was used as the source of excitation. Copolymer samples exhibited reverse saturable absorption (RSA) process. The nonlinear refraction studies depict that the copolymers exhibit self-defocusing property. The estimated values of βeff, n2 and χ(3) were found to be of the order of 10-2 cm/W, 10-5 esu and 10-7 esu respectively. Self-diffraction rings were observed due to refractive index change when exposed to the laser beam. A good optical limiting and clamping of power of ∼0.9 mW and ∼0.05 mW was observed. Therefore, copolymers of aniline emerge as a potential candidate for photonic device applications.
Optical soliton solutions for two coupled nonlinear Schroedinger systems via Darboux transformation
International Nuclear Information System (INIS)
Zhang Haiqiang; Li Juan; Xu Tao; Zhang Yaxing; Hu Wei; Tian Bo
2007-01-01
In nonlinear optical fibers, the vector solitons can be governed by the systems of coupled nonlinear Schroedinger from polarized optical waves in an isotropic medium. Based on the Ablowitz-Kaup-Newell-Segur technology, the Darboux transformation method is successfully applied to two coupled nonlinear Schroedinger systems. With the help of symbolic computation, the bright vector one- and two-soliton solutions including one-peak and two-peak solitons are further constructed via the iterative algorithm of Darboux transformation. Through the figures for several sample solutions, the stable propagation and elastic collisions for these kinds of bright vector solitons are discussed and the possible applications are pointed out in optical communications and relevant optical experiments.In addition, the conserved quantities of such two systems, i.e., the energy, momentum and Hamiltonian, are also presented
Optical super-resolution effect induced by nonlinear characteristics of graphene oxide films
Zhao, Yong-chuang; Nie, Zhong-quan; Zhai, Ai-ping; Tian, Yan-ting; Liu, Chao; Shi, Chang-kun; Jia, Bao-hua
2018-01-01
In this work, we focus on the optical super-resolution effect induced by strong nonlinear saturation absorption (NSA) of graphene oxide (GO) membranes. The third-order optical nonlinearities are characterized by the canonical Z-scan technique under femtosecond laser (wavelength: 800 nm, pulse width: 100 fs) excitation. Through controlling the applied femtosecond laser energy, NSA of the GO films can be tuned continuously. The GO film is placed at the focal plane as a unique amplitude filter to improve the resolution of the focused field. A multi-layer system model is proposed to present the generation of a deep sub-wavelength spot associated with the nonlinearity of GO films. Moreover, the parameter conditions to achieve the best resolution (˜λ/6) are determined entirely. The demonstrated results here are useful for high density optical recoding and storage, nanolithography, and super-resolution optical imaging.
A nonlinear plasmonic resonator for three-state all-optical switching
Amin, Muhammad; Farhat, Mohamed; Bagci, Hakan
2014-01-01
A nonlinear plasmonic resonator design is proposed for three-state all-optical switching at frequencies including near infrared and lower red parts of the spectrum. The tri-stable response required for three-state operation is obtained by enhancing nonlinearities of a Kerr medium through multiple (higher order) plasmons excited on resonator's metallic surfaces. Indeed, simulations demonstrate that exploitation of multiple plasmons equips the proposed resonator with a multi-band tri-stable response, which cannot be obtained using existing nonlinear plasmonic devices that make use of single mode Lorentzian resonances. Multi-band three-state optical switching that can be realized using the proposed resonator has potential applications in optical communications and computing. © 2014 Optical Society of America.
Natural Silk as a Photonics Component: a Study on Its Light Guiding and Nonlinear Optical Properties
Kujala, Sami; Mannila, Anna; Karvonen, Lasse; Kieu, Khanh; Sun, Zhipei
2016-01-01
Silk fibers are expected to become a pathway to biocompatible and bioresorbable waveguides, which could be used to deliver localized optical power for various applications, e.g., optical therapy or imaging inside living tissue. Here, for the first time, the linear and nonlinear optical properties of natural silk fibers have been studied. The waveguiding properties of silk fibroin of largely unprocessed Bombyx mori silkworm silk are assessed using two complementary methods, and found to be on ...
Multiphase Weakly Nonlinear Geometric Optics for Schrödinger Equations
Carles, Ré mi; Dumas, Eric; Sparber, Christof
2010-01-01
We describe and rigorously justify the nonlinear interaction of highly oscillatory waves in nonlinear Schrödinger equations, posed on Euclidean space or on the torus. Our scaling corresponds to a weakly nonlinear regime where the nonlinearity affects the leading order amplitude of the solution, but does not alter the rapid oscillations. We consider initial states which are superpositions of slowly modulated plane waves, and use the framework of Wiener algebras. A detailed analysis of the corresponding nonlinear wave mixing phenomena is given, including a geometric interpretation of the resonance structure for cubic nonlinearities. As an application, we recover and extend some instability results for the nonlinear Schrödinger equation on the torus in negative order Sobolev spaces. © 2010 Society for Industrial and Applied Mathematics.
Hosseini, Mahdi
Our ability to engineer quantum states of light and matter has significantly advanced over the past two decades, resulting in the production of both Gaussian and non-Gaussian optical states. The resulting tailored quantum states enable quantum technologies such as quantum optical communication, quantum sensing as well as quantum photonic computation. The strong nonlinear light-atom interaction is the key to deterministic quantum state preparation and quantum photonic processing. One route to enhancing the usually weak nonlinear light-atom interactions is to approach the regime of cavity quantum electrodynamics (cQED) interaction by means of high finesse optical resonators. I present results from the MIT experiment of large conditional cross-phase modulation between a signal photon, stored inside an atomic quantum memory, and a control photon that traverses a high-finesse optical cavity containing the atomic memory. I also present a scheme to probabilistically change the amplitude and phase of a signal photon qubit to, in principle, arbitrary values by postselection on a control photon that has interacted with that state. Notably, small changes of the control photon polarization measurement basis by few degrees can substantially change the amplitude and phase of the signal state. Finally, I present our ongoing effort at Purdue to realize similar peculiar quantum phenomena at the single photon level on chip scale photonic systems.
Harnessing mode-selective nonlinear optics for on-chip multi-channel all-optical signal processing
Directory of Open Access Journals (Sweden)
Ming Ma
2016-11-01
Full Text Available All-optical signal processing based on nonlinear optical effects allows for the realization of important functions in telecommunications including wavelength conversion, optical multiplexing/demultiplexing, Fourier transformation, and regeneration, amongst others, on ultrafast time scales to support high data rate transmission. In integrated photonic subsystems, the majority of all-optical signal processing systems demonstrated to date typically process only a single channel at a time or perform a single processing function, which imposes a serious limitation on the functionality of integrated solutions. Here, we demonstrate how nonlinear optical effects can be harnessed in a mode-selective manner to perform simultaneous multi-channel (two and multi-functional optical signal processing (i.e., regenerative wavelength conversion in an integrated silicon photonic device. This approach, which can be scaled to a higher number of channels, opens up a new degree of freedom for performing a broad range of multi-channel nonlinear optical signal processing functions using a single integrated photonic device.
Directory of Open Access Journals (Sweden)
Ryu Jiheun
2015-01-01
Full Text Available During the research using fluorescence-tagged or auto-fluorescence molecules, meaningful information is often buried deep inside the tissue, not its surface. Therefore, especially in the field of biomedical imaging, acquiring optically sectioned images from deep inside the tissue is very important. As well know already, confocal laser scanning microscopy (the most well-known optical sectioning microscopy gives axially-resolved fluorescence information using the physical background blocking component called pinhole. However, the axial range of imaging is practically limited due to such optical phenomena as the light scattered and absorbed in the tissue. However, nonlinear optical microscopy (e.g. Multiphoton microscopy, harmonic generation microscopy, coherent anti-Stokes Raman spectroscopy realized by the development of ultrafast light sources has been used for visualizing various tissues, especially in vivo, because of their low sensitivity to the limitation caused by the scattering and the absorption of light. Although nonlinear optical microscopy gives deep tissue image, it is not easy for many researcher to build customized nonlinear system. Here, we introduce an easy and simple way designing and developing such nonlinear optical microscope with upright or inverted epi-illumination platform using commercial optical components only.
Effects of high light intensities on the optical Kerr nonlinearity of semiconducting polymers
International Nuclear Information System (INIS)
Charra, Fabrice
1990-01-01
Experimental investigations, in the picosecond time scale, of the Kerr type optical nonlinearity (or pump and probe) are presented. The nonlinear molecules semiconducting polymers of the type poly-diacetylene. The degenerate case (pump and probe at the same frequency) has been studied by four wave mixing at 1064 nm, in the configuration of phase conjugation. It is shown that the response is dominated by high orders of nonlinearity. The results are analysed in terms of two photon resonance. The non-degenerate case is studied by two wave mixing or in the optical Kerr gate experiment. The optical Stark effect and the differential spectra of photoinduced species are analysed. Two photon excitations at 1064 nm and one photon excitations at 532 nm are compared. A consequence of the mechanism of the nonlinearity is the possibility of generating phase conjugate waves at double frequency. The theoretical analysis and the experimental demonstration of this process are presented. The experiment is only sensitive to nonlinearities of the fifth order or more and thus allows to clarify its origins and dynamics. Finally, quantum modelling and calculations of the nonlinear optical responses, developed for the interpretations of the above experiments, are presented. (author) [fr
An analog model for quantum lightcone fluctuations in nonlinear optics
International Nuclear Information System (INIS)
Ford, L.H.; De Lorenci, V.A.; Menezes, G.; Svaiter, N.F.
2013-01-01
We propose an analog model for quantum gravity effects using nonlinear dielectrics. Fluctuations of the spacetime lightcone are expected in quantum gravity, leading to variations in the flight times of pulses. This effect can also arise in a nonlinear material. We propose a model in which fluctuations of a background electric field, such as that produced by a squeezed photon state, can cause fluctuations in the effective lightcone for probe pulses. This leads to a variation in flight times analogous to that in quantum gravity. We make some numerical estimates which suggest that the effect might be large enough to be observable. - Highlights: ► Lightcone fluctuations, quantum fluctuations of the effective speed of light, are a feature of quantum gravity. ► Nonlinear dielectrics have a variable speed of light, analogous to the effects of gravity. ► Fluctuating electric fields create the effect of lightcone fluctuations in a nonlinear material. ► We propose to use squeezed light in a nonlinear material as an analog model of lightcone fluctuations. ► Variation in the speed of propagation of pulses is the observational signature of lightcone fluctuations.
Linear and nonlinear optical properties of Sb-doped GeSe2 thin films
Zhang, Zhen-Ying; Chen, Fen; Lu, Shun-Bin; Wang, Yong-Hui; Shen, Xiang; Dai, Shi-Xun; Nie, Qiu-Hua
2015-06-01
Sb-doped GeSe2 chalcogenide thin films are prepared by the magnetron co-sputtering method. The linear optical properties of as-deposited films are derived by analyzing transmission spectra. The refractive index rises and the optical band gap decreases from 2.08 eV to 1.41 eV with increasing the Sb content. X-ray photoelectron spectra further confirm the formation of a covalent Sb-Se bond. The third-order nonlinear optical properties of thin films are investigated under femtosecond laser excitation at 800 nm. The results show that the third-order nonlinear optical properties are enhanced with increasing the concentration of Sb. The nonlinear refraction indices of these thin films are measured to be on the order of 10-18 m2/W with a positive sign and the nonlinear absorption coefficients are obtained to be on the order of 10-10 m/W. These excellent properties indicate that Sb-doped Ge-Se films have a good prospect in the applications of nonlinear optical devices. Project supported by the National Key Basic Research Program of China (Grant No. 2012CB722703), the National Natural Science Foundation of China (Grant No. 61377061), the Young Leaders of Academic Climbing Project of the Education Department of Zhejiang Province, China (Grant No. pd2013092), the Program for Innovative Research Team of Ningbo City, China (Grant No. 2009B217), and the K. C. Wong Magna Fund in Ningbo University, China.
International Nuclear Information System (INIS)
Pramodini, S; Poornesh, P; Sudhakar, Y N; SelvaKumar, M
2014-01-01
We present the synthesis and characterization of third-order optical nonlinearity and optical limiting of the conducting polymers poly (aniline-co-o-anisidine) and poly (aniline-co-pyrrole). Nonlinear optical studies were carried out by employing the z-scan technique using a He–Ne laser operating in continuous wave mode at 633 nm. The copolymers exhibited a reverse saturable absorption process and self-defocusing properties under the experimental conditions. The estimated values of β eff , n 2 and χ (3) were found to be of the order of 10 −2 cm W −1 , 10 -5 esu and 10 −7 esu respectively. Self-diffraction rings were observed due to refractive index change when exposed to the laser beam. The copolymers possess a lower limiting threshold and clamping level, which is essential to a great extent for power limiting devices. Therefore, copolymers of aniline emerge as a potential candidate for nonlinear optical device applications. (paper)
Dynamics of Nonlinear Excitation of the High-Order Mode in a Single-Mode Step-Index Optical Fiber
Burdin, V.; Bourdine, A.
2018-04-01
This work is concerned with approximate model of higher-order mode nonlinear excitation in a singlemode silica optical fiber. We present some results of simulation for step-index optical fiber under femtosecond optical pulse launching, which confirm ability of relatively stable higher-order mode excitation in such singlemode optical fiber over sufficiently narrow range of launched optical power variation.
Nonlinear interaction of colliding beams in particle storage rings
International Nuclear Information System (INIS)
Herrera, J.C.; Month, M.
1979-01-01
When two beams of high energy particles moving in opposite directions are brought into collision, a large amount of energy is available for the production of new particles. However to obtain a sufficiently high event rate for rare processes, such as the production of the intermediate vector boson (Z 0 and W +- ), large beam currents are also required. Under this circumstance, the high charge density of one beam results in a classical electromagnetic interaction on the particles in the other beam. This very nonlinear space charge force, caled the beam-beam force, limits the total circulating charge and, thereby, the ultimate performance of the colliding ring system. The basic nature of the beam-beam force is discussed, indicating how it is quite different in the case of continuous beams, which cross each other at an angle as compared to the case of bunched beams which collide head-on. Some experimental observations on the beam-beam interaction in proton-proton and electron-positron beams are then reviewed and interpreted. An important aspect of the beam-beam problem in storage rings is to determine at what point in the analysis of the particle dynamics is it relevant to bring in the concepts of stochasticity, slow diffusion, and resonance overlap. These ideas are briefly discussed
A test to evaluation non-linear soil structure interaction
International Nuclear Information System (INIS)
Hagiwara, T.; Kitada, Y.
2005-01-01
JNES is planning a new project to study non-linear soil-structure interaction (SSI) effect under large earthquake ground motions equivalent to and/or over a design earthquake ground motion of S2. Concerning the SSI test, it is pointed out that handling of the scale effect of the specimen taking into account the surrounding soil on the earthquake response evaluation to the actual structure is essential issue for the scaled model test. Thus, for the test, the largest specimen possible and the biggest input motion possible are necessary. Taking into account the above issues, new test methodology, which utilizes artificial earthquake ground motion, is considered desirable if it can be performed at a realistic cost. With this motivation, we have studied the test methodology which applying blasting power as for a big earthquake ground motion. The information from a coalmine company in the U.S.A. indicates that the works performed in the surface coalmine to blast a rock covering a coal layer generates a big artificial ground motion, which is similar to earthquake ground motion. Application of this artificial earthquake ground motion for the SSI test is considered very promising because the blasting work is carried out periodically for mining coal so that we can apply artificial motions generated by the work if we construct a building model at a closed point to the blasting work area. The major purposes of the test are to understand (a) basic earthquake response characteristics of a Nuclear Power Plant (NPP) reactor building when a large earthquake strikes the NPP site and (b) nonlinear characteristics of SSI phenomenon during a big earthquake. In the paper of ICONE-13, we will introduce the test method and basic characteristics of measured artificial ground motions generated by the blasting works on an actual site. (authors)
Nonlinear optical microscopy for histology of fresh normal and cancerous pancreatic tissues.
Directory of Open Access Journals (Sweden)
Wenyan Hu
Full Text Available BACKGROUND: Pancreatic cancer is a lethal disease with a 5-year survival rate of only 1-5%. The acceleration of intraoperative histological examination would be beneficial for better management of pancreatic cancer, suggesting an improved survival. Nonlinear optical methods based on two-photon excited fluorescence (TPEF and second harmonic generation (SHG of intrinsic optical biomarkers show the ability to visualize the morphology of fresh tissues associated with histology, which is promising for real-time intraoperative evaluation of pancreatic cancer. METHODOLOGY/PRINCIPAL FINDINGS: In order to investigate whether the nonlinear optical imaging methods have the ability to characterize pancreatic histology at cellular resolution, we studied different types of pancreatic tissues by using label-free TPEF and SHG. Compared with other routine methods for the preparation of specimens, fresh tissues without processing were found to be most suitable for nonlinear optical imaging of pancreatic tissues. The detailed morphology of the normal rat pancreas was observed and related with the standard histological images. Comparatively speaking, the preliminary images of a small number of chemical-induced pancreatic cancer tissues showed visible neoplastic differences in the morphology of cells and extracellular matrix. The subcutaneous pancreatic tumor xenografts were further observed using the nonlinear optical microscopy, showing that most cells are leucocytes at 5 days after implantation, the tumor cells begin to proliferate at 10 days after implantation, and the extracellular collagen fibers become disordered as the xenografts grow. CONCLUSIONS/SIGNIFICANCE: In this study, nonlinear optical imaging was used to characterize the morphological details of fresh pancreatic tissues for the first time. We demonstrate that it is possible to provide real-time histological evaluation of pancreatic cancer by the nonlinear optical methods, which present an
Nonlinear localized modes in dipolar Bose–Einstein condensates in two-dimensional optical lattices
International Nuclear Information System (INIS)
Rojas-Rojas, Santiago; Naether, Uta; Delgado, Aldo; Vicencio, Rodrigo A.
2016-01-01
Highlights: • We study discrete two-dimensional breathers in dipolar Bose–Einstein Condensates. • Important differences in the properties of three fundamental modes are found. • Norm threshold for existence of 2D breathers varies with dipolar interaction. • The Effective Potential Method is implemented for stability analysis. • Uncommon mobility of 2D discrete solitons is observed. - Abstract: We analyze the existence and properties of discrete localized excitations in a Bose–Einstein condensate loaded into a periodic two-dimensional optical lattice, when a dipolar interaction between atoms is present. The dependence of the Number of Atoms (Norm) on the energy of solutions is studied, along with their stability. Two important features of the system are shown, namely, the absence of the Norm threshold required for localized solutions to exist in finite 2D systems, and the existence of regions in the parameter space where two fundamental solutions are simultaneously unstable. This feature enables mobility of localized solutions, which is an uncommon feature in 2D discrete nonlinear systems. With attractive dipolar interaction, a non-trivial behavior of the Norm dependence is obtained, which is well described by an analytical model.
Nonlinear localized modes in dipolar Bose–Einstein condensates in two-dimensional optical lattices
Energy Technology Data Exchange (ETDEWEB)
Rojas-Rojas, Santiago, E-mail: srojas@cefop.cl [Center for Optics and Photonics and MSI-Nucleus on Advanced Optics, Universidad de Concepción, Casilla 160-C, Concepción (Chile); Departamento de Física, Universidad de Concepción, Casilla 160-C, Concepción (Chile); Naether, Uta [Instituto de Ciencia de Materiales de Aragón and Departamento de Física de la Materia Condensada, CSIC-Universidad de Zaragoza, 50009 Zaragoza (Spain); Delgado, Aldo [Center for Optics and Photonics and MSI-Nucleus on Advanced Optics, Universidad de Concepción, Casilla 160-C, Concepción (Chile); Departamento de Física, Universidad de Concepción, Casilla 160-C, Concepción (Chile); Vicencio, Rodrigo A. [Center for Optics and Photonics and MSI-Nucleus on Advanced Optics, Universidad de Concepción, Casilla 160-C, Concepción (Chile); Departamento de Física, Facultad de Ciencias, Universidad de Chile, Santiago (Chile)
2016-09-16
Highlights: • We study discrete two-dimensional breathers in dipolar Bose–Einstein Condensates. • Important differences in the properties of three fundamental modes are found. • Norm threshold for existence of 2D breathers varies with dipolar interaction. • The Effective Potential Method is implemented for stability analysis. • Uncommon mobility of 2D discrete solitons is observed. - Abstract: We analyze the existence and properties of discrete localized excitations in a Bose–Einstein condensate loaded into a periodic two-dimensional optical lattice, when a dipolar interaction between atoms is present. The dependence of the Number of Atoms (Norm) on the energy of solutions is studied, along with their stability. Two important features of the system are shown, namely, the absence of the Norm threshold required for localized solutions to exist in finite 2D systems, and the existence of regions in the parameter space where two fundamental solutions are simultaneously unstable. This feature enables mobility of localized solutions, which is an uncommon feature in 2D discrete nonlinear systems. With attractive dipolar interaction, a non-trivial behavior of the Norm dependence is obtained, which is well described by an analytical model.
Wang, Aijian; Yu, Wang; Huang, Zhipeng; Zhou, Feng; Song, Jingbao; Song, Yinglin; Long, Lingliang; Cifuentes, Marie P.; Humphrey, Mark G.; Zhang, Long; Shao, Jianda; Zhang, Chi
2016-03-01
Reduced graphene oxide (RGO)-porphyrin (TPP) nanohybrids (RGO-TPP 1 and RGO-TPP 2) were prepared by two synthetic routes that involve functionalization of the RGO using diazonium salts. The microscopic structures, morphology, photophysical properties and nonlinear optical performance of the resultant RGO-TPP nanohybrids were investigated. The covalent bonding of the porphyrin-functionalized-RGO nanohybrid materials was confirmed by Fourier transform infrared spectroscopy, Raman spectroscopy, X-ray photoelectron spectroscopy, transmission electron microscopy, and thermogravimetric analysis. Attachment of the porphyrin units to the surface of the RGO by diazotization significantly improves the solubility and ease of processing of these RGO-based nanohybrid materials. Ultraviolet/visible absorption and steady-state fluorescence studies indicate considerable π-π interactions and effective photo-induced electron and/or energy transfer between the porphyrin moieties and the extended π-system of RGO. The nonlinear optical properties of RGO-TPP 1 and RGO-TPP 2 were investigated by open-aperture Z-scan measurements at 532 nm with both 4 ns and 21 ps laser pulses, the results showing that the chemical nanohybrids exhibit improved nonlinear optical properties compared to those of the benchmark material C60, and the constituent RGO or porphyrins.
Spectral dependence of third-order nonlinear optical properties in InN
International Nuclear Information System (INIS)
Ahn, H.; Lee, M.-T.; Chang, Y.-M.
2014-01-01
We report on the nonlinear optical properties of InN measured in a wide near-infrared spectral range with the femtosecond Z-scan technique. The above-bandgap nonlinear absorption in InN is found to originate from the saturation of absorption by the band-state-filling and its cross-section increases drastically near the bandgap energy. With below-bandgap excitation, the nonlinear absorption undergoes a transition from saturation absorption (SA) to reverse-SA (RSA), attributed to the competition between SA of band-tail states and two-photon-related RSA. The measured large nonlinear refractive index of the order of 10 −10 cm 2 /W indicates InN as a potential material for all-optical switching and related applications
Ultrafast Relaxation Dynamics of the Optical Nonlinearity in Nanometric Gold Particles
International Nuclear Information System (INIS)
Puech, K.; Blau, W.J.
2001-01-01
Measurements of the resonantly enhanced, third-order nonlinear optical properties of gold nanostructures exhibiting reduced charge-carrier mobility in three dimensions were performed with a number of ultrafast nonlinear optical techniques. The size of the particles investigated was varied between 5 and 40 nm. The magnitude of the nonlinear susceptibility is of the order of 5.10 -16 m 2 V -2 at resonance and an order of magnitude lower off-resonance. The response time of the nonlinearity is found to be extremely fast and could not be resolved in the experiments undertaken here. The only statement that can be made in this regard is that the phase relaxation time is of the order of or less than 20 fs while the energy relaxation time is of the order of or less than 75 fs
Rational solitons in deep nonlinear optical Bragg grating
Alatas, H.; Iskandar, A.A.; Tjia, M.O.; Valkering, T.P.
2006-01-01
We have examined the rational solitons in the Generalized Coupled Mode model for a deep nonlinear Bragg grating. These solitons are the degenerate forms of the ordinary solitons and appear at the transition lines in the parameter plane. A simple formulation is presented for the investigation of the
Extreme non-linear elasticity and transformation optics
DEFF Research Database (Denmark)
Gersborg, Allan Roulund; Sigmund, Ole
2010-01-01
realizations correspond to minimizers of elastic energy potentials for extreme values of the mechanical Poisson's ratio ν . For TE (Hz) polarized light an incompressible transformation ν = 1/2 is ideal and for TM (E z) polarized light one should use a compressible transformation with negative Poissons's ratio......Transformation optics is a powerful concept for designing novel optical components such as high transmission waveguides and cloaking devices. The selection of specific transformations is a non-unique problem. Here we reveal that transformations which allow for all dielectric and broadband optical...... ν = -1. For the TM polarization the mechanical analogy corresponds to a modified Liao functional known from the transformation optics literature. Finally, the analogy between ideal transformations and solid mechanical material models automates and broadens the concept of transformation optics...
Nonlinear optical properties of TeO$_2$ crystalline phases from first principles
Berkaine, Nabil; Orhan, Emmanuelle; Masson, Olivier; Thomas, Philippe; Junquera, Javier
2010-01-01
We have computed second and third nonlinear optical susceptibilities of two crystalline bulk tellurium oxide polymorphs: $\\alpha$-TeO$_{2}$ (the most stable crystalline bulk phase) and $\\gamma$-TeO$_{2}$ (the crystalline phase that ressembles the more to the glass phase. Third order nonlinear susceptibilities of the crystalline phases are two orders of magnitude larger than $\\alpha$-SiO$_{2}$ cristoballite, thus extending the experimental observations on glasses to the case of crystalline com...
Yamuna, R.; Ramakrishnan, S.; Dhara, Keerthy; Devi, R.; Kothurkar, Nikhil K.; Kirubha, E.; Palanisamy, P. K.
2013-01-01
The synthesis of a porphyrin-graphene oxide hybrid (GO-TAP) was carried out by covalently functionalizing graphene oxide (GO) with 5,10,15,20 mesotetra (4-aminophenyl) porphyrin (TAP) through an amide linkage. The GO-TAP hybrid has been characterized by Fourier transform infrared spectroscopy, X-ray photoelectron spectroscopy, and UV-visible spectroscopy. The peak intensity of the Soret band of the material was suppressed compared to neat TAP. This indicates a strong interaction between the electronic energy level of TAP and GO in the GO-TAP hybrid. The functionalization of GO with TAP significantly improved its solubility and dispersion stability in organic solvents. Scanning electron micrographs reveal that the hybrid was found to be similar to the unmodified GO but slightly more wrinkled. Transmission electron micrographs also demonstrate that GO sheet in the hybrid is more wrinkled with some dark spot due to functionalization. Atomic force microscopy results also reveal that the TAP functionalization increases the thickness of GO sheet to 2.0-3.0 nm from 1.2 to 1.8 nm. We observed improved nonlinear optical and optical limiting properties for the hybrid compared to both graphene oxide and porphyrin. GO-TAP shows fluorescence quenching compared with porphyrin, indicating excellent electron and/or energy transfer to GO from TAP. Thermogravimetric analysis confirms that the GO-TAP hybrid has outstanding thermal stability.
International Nuclear Information System (INIS)
Yamuna, R.; Ramakrishnan, S.; Dhara, Keerthy; Devi, R.; Kothurkar, Nikhil K.; Kirubha, E.; Palanisamy, P. K.
2013-01-01
The synthesis of a porphyrin–graphene oxide hybrid (GO–TAP) was carried out by covalently functionalizing graphene oxide (GO) with 5,10,15,20 mesotetra (4-aminophenyl) porphyrin (TAP) through an amide linkage. The GO–TAP hybrid has been characterized by Fourier transform infrared spectroscopy, X-ray photoelectron spectroscopy, and UV–visible spectroscopy. The peak intensity of the Soret band of the material was suppressed compared to neat TAP. This indicates a strong interaction between the electronic energy level of TAP and GO in the GO–TAP hybrid. The functionalization of GO with TAP significantly improved its solubility and dispersion stability in organic solvents. Scanning electron micrographs reveal that the hybrid was found to be similar to the unmodified GO but slightly more wrinkled. Transmission electron micrographs also demonstrate that GO sheet in the hybrid is more wrinkled with some dark spot due to functionalization. Atomic force microscopy results also reveal that the TAP functionalization increases the thickness of GO sheet to 2.0–3.0 nm from 1.2 to 1.8 nm. We observed improved nonlinear optical and optical limiting properties for the hybrid compared to both graphene oxide and porphyrin. GO–TAP shows fluorescence quenching compared with porphyrin, indicating excellent electron and/or energy transfer to GO from TAP. Thermogravimetric analysis confirms that the GO–TAP hybrid has outstanding thermal stability.
Robust Numerical Methods for Nonlinear Wave-Structure Interaction in a Moving Frame of Reference
DEFF Research Database (Denmark)
Kontos, Stavros; Lindberg, Ole
This project is focused on improving the state of the art for predicting the interaction between nonlinear ocean waves and marine structures. To achieve this goal, a flexible order finite difference potential flow solver has been extended to calculate for fully nonlinear wave-structure interaction...
Ultra-fast dynamics in the nonlinear optical response of silver nanoprism ordered arrays.
Sánchez-Esquivel, Héctor; Raygoza-Sanchez, Karen Y; Rangel-Rojo, Raúl; Kalinic, Boris; Michieli, Niccolò; Cesca, Tiziana; Mattei, Giovanni
2018-03-15
In this work we present the study of the ultra-fast dynamics of the nonlinear optical response of a honeycomb array of silver triangular nanoprisms, performed using a femtosecond pulsed laser tuned with the dipolar surface plasmon resonance of the nanoarray. Nonlinear absorption and refraction, and their time-dependence, were explored using the z-scan and time-resolved excite-probe techniques. Nonlinear absorption is shown to change sign with the input irradiance and the behavior was explained on the basis of a three-level model. The response time was determined to be in the picosecond regime. A technique based on a variable frequency chopper was also used in order to discriminate the thermal and electronic contributions to the nonlinearity, which were found to have opposite signs. All these findings propel the investigated nanoprism arrays as good candidates for applications in advanced ultra-fast nonlinear nanophotonic devices.
Investigation of nonlinear optical properties of various organic materials by the Z-scan method
Ganeev, R. A.; Boltaev, G. S.; Tugushev, R. I.; Usmanov, T.
2012-06-01
We have studied the nonlinear optical properties of various organic materials (vegetable oil, juice, wine, cognac, Coca-Cola and Fanta drinks, Nescafé coffee, tea, gasoline, clock oil, glycerol, and polyphenyl ether) that are used in everyday life. Their nonlinearities have been studied by the Z-scan method in the near-IR and visible spectral ranges. We have shown that the majority of samples possess a nonlinear absorption; however, some of the studied materials show a strong saturated absorption and nonlinear refraction. Red wine and glycerol proved to be the most interesting materials. For these samples, we have observed a change in the sign of the nonlinear absorption with increasing laser intensity, which was attributed to the competition between two-photon absorption and saturated absorption.
Measurements of nonlinear optical properties of PVDF/ZnO using Z-scan technique
Energy Technology Data Exchange (ETDEWEB)
Shanshool, Haider Mohammed, E-mail: haidshan62@gmail.com [Ministry of Science and Technology, Baghdad (Iraq); Yahaya, Muhammad [School of Applied Physics, Faculty of Science and Technology, Universiti Kebangsaan Malaysia, Selangor (Malaysia); Yunus, Wan Mahmood Mat [Department of Physics, Faculty of Science, University Putra Malaysia, Serdang (Malaysia); Abdullah, Ibtisam Yahya [Department of Physics, College of Science, University of Mosul, Mosul (Iraq)
2015-10-15
The nonlinear optical properties of ZnO nanoparticles dispersed in poly (vinylidene fluoride) (PVDF) polymer are investigated. PVDF/ZnO nanocomposites were prepared by mixing different concentrations of ZnO nanoparticles, as the filler, with PVDF, as the polymer matrix, using casting method. Acetone was used as a solvent for the polymer. FTIR spectra of the samples were analyzed thus confirming the formation of α and β phases. The absorbance spectra of the samples were obtained, thereby showing high absorption in the UV region. The linear absorption coefficient was calculated. The single-beam Z-scan technique was used to measure the nonlinear refractive index and the nonlinear absorption coefficient of the PVDF/ZnO nanocomposite samples. We observed that the nonlinear refractive index is in the order of 10{sup -13} cm{sup 2}/W with the negative sign, whereas the nonlinear absorption coefficient is in the order of 10{sup -8} cm/W. (author)
Xu, Tianhua; Karanov, Boris; Shevchenko, Nikita A; Lavery, Domaniç; Liga, Gabriele; Killey, Robert I; Bayvel, Polina
2017-10-11
Nyquist-spaced transmission and digital signal processing have proved effective in maximising the spectral efficiency and reach of optical communication systems. In these systems, Kerr nonlinearity determines the performance limits, and leads to spectral broadening of the signals propagating in the fibre. Although digital nonlinearity compensation was validated to be promising for mitigating Kerr nonlinearities, the impact of spectral broadening on nonlinearity compensation has never been quantified. In this paper, the performance of multi-channel digital back-propagation (MC-DBP) for compensating fibre nonlinearities in Nyquist-spaced optical communication systems is investigated, when the effect of signal spectral broadening is considered. It is found that accounting for the spectral broadening effect is crucial for achieving the best performance of DBP in both single-channel and multi-channel communication systems, independent of modulation formats used. For multi-channel systems, the degradation of DBP performance due to neglecting the spectral broadening effect in the compensation is more significant for outer channels. Our work also quantified the minimum bandwidths of optical receivers and signal processing devices to ensure the optimal compensation of deterministic nonlinear distortions.
Synthesis, characterization and non-linear optical response of organophilic carbon dots
Bourlinos, Athanasios B.; Karakassides, Michael A.; Kouloumpis, Antonios; Gournis, Dimitrios; Bakandritsos, Aristides; Papagiannouli, Irene; Aloukos, Panagiotis; Couris, Stelios; Hola, Katerina; Zboril, Radek; Krysmann, Marta; Giannelis, Emmanuel P.
2013-01-01
For the first time ever we report the nonlinear optical (NLO) properties of carbon dots (C-dots). The C-dots for these experiments were synthesized by mild pyrolysis of lauryl gallate. The resulting C-dots bear lauryl chains and, hence, are highly dispersible in polar organic solvents, like chloroform. Dispersions in CHCl3 show significant NLO response. Specifically, the C-dots show negative nonlinear absorption coefficient and negative nonlinear refraction. Using suspensions with different concentrations these parameters are quantified and compared to those of fullerene a well-known carbon molecule with proven NLO response. © 2013 Elsevier Ltd. All rights reserved.
Synthesis, characterization and non-linear optical response of organophilic carbon dots
Bourlinos, Athanasios B.
2013-09-01
For the first time ever we report the nonlinear optical (NLO) properties of carbon dots (C-dots). The C-dots for these experiments were synthesized by mild pyrolysis of lauryl gallate. The resulting C-dots bear lauryl chains and, hence, are highly dispersible in polar organic solvents, like chloroform. Dispersions in CHCl3 show significant NLO response. Specifically, the C-dots show negative nonlinear absorption coefficient and negative nonlinear refraction. Using suspensions with different concentrations these parameters are quantified and compared to those of fullerene a well-known carbon molecule with proven NLO response. © 2013 Elsevier Ltd. All rights reserved.
Defect solitons in saturable nonlinearity media with parity-time symmetric optical lattices
Energy Technology Data Exchange (ETDEWEB)
Hu, Sumei [Department of Physics, Guangdong University of Petrochemical Technology, Maoming 525000 (China); Laboratory of Nanophotonic Functional Materials and Devices, South China Normal University, Guangzhou 510631 (China); Hu, Wei, E-mail: huwei@scnu.edu.cn [Laboratory of Nanophotonic Functional Materials and Devices, South China Normal University, Guangzhou 510631 (China)
2013-11-15
We reported the existence and stability of defect solitons in saturable nonlinearity media with parity-time (PT) symmetric optical lattices. Families of fundamental and dipole solitons are found in the semi-infinite gap and the first gap. The power of solitons increases with the increasing of the propagation constant and saturation parameter. The existence areas of fundamental and dipole solitons shrink with the growth of saturation parameter. The instability of dipole solitons for positive and no defect induced by the imaginary part of PT symmetric potentials can be suppressed by the saturation nonlinearity, but for negative defect it cannot be suppressed by the saturation nonlinearity.
Nonlinear tunneling of optical soliton in 3 coupled NLS equation with symbolic computation
Energy Technology Data Exchange (ETDEWEB)
Mani Rajan, M.S., E-mail: senthilmanirajanofc@gmail.com [Department of Physics, Anna University, Madurai Region, Ramanathapuram (India); Mahalingam, A. [Department of Physics, Anna University, Chennai - 600 025 (India); Uthayakumar, A. [Department of Physics, Presidency College, Chennai - 600 005 (India)
2014-07-15
We investigated the soliton solution for N coupled nonlinear Schrödinger (CNLS) equations. These equations are coupled due to the cross-phase-modulation (CPM). Lax pair of this system is obtained via the Ablowitz–Kaup–Newell–Segur (AKNS) scheme and the corresponding Darboux transformation is constructed to derive the soliton solution. One and two soliton solutions are generated. Using two soliton solutions of 3 CNLS equation, nonlinear tunneling of soliton for both with and without exponential background has been discussed. Finally cascade compression of optical soliton through multi-nonlinear barrier has been discussed. The obtained results may have promising applications in all-optical devices based on optical solitons, study of soliton propagation in birefringence fiber systems and optical soliton with distributed dispersion and nonlinearity management. -- Highlights: •We consider the nonlinear tunneling of soliton in birefringence fiber. •3-coupled NLS (CNLS) equation with variable coefficients is considered. •Two soliton solutions are obtained via Darboux transformation using constructed Lax pair. •Soliton tunneling through dispersion barrier and well are investigated. •Finally, cascade compression of soliton has been achieved.
Inan, B.; Lee, S.C.J.; Randel, S.; Neokosmidis, L.; Koonen, A.M.J.; Walewski, J.
2009-01-01
The nonlinear dependence of the optical power from white LEDs on the applied driving current and its impact on discrete-multitone modulation was investigated by use of numerical simulations for the case of optical wireless communications.
Perspective: Quantum Hamiltonians for optical interactions
Andrews, David L.; Jones, Garth A.; Salam, A.; Woolley, R. Guy
2018-01-01
The multipolar Hamiltonian of quantum electrodynamics is extensively employed in chemical and optical physics to treat rigorously the interaction of electromagnetic fields with matter. It is also widely used to evaluate intermolecular interactions. The multipolar version of the Hamiltonian is commonly obtained by carrying out a unitary transformation of the Coulomb gauge Hamiltonian that goes by the name of Power-Zienau-Woolley (PZW). Not only does the formulation provide excellent agreement with experiment, and versatility in its predictive ability, but also superior physical insight. Recently, the foundations and validity of the PZW Hamiltonian have been questioned, raising a concern over issues of gauge transformation and invariance, and whether observable quantities obtained from unitarily equivalent Hamiltonians are identical. Here, an in-depth analysis of theoretical foundations clarifies the issues and enables misconceptions to be identified. Claims of non-physicality are refuted: the PZW transformation and ensuing Hamiltonian are shown to rest on solid physical principles and secure theoretical ground.
Korjik, M. V.; Buganov, O.; Fedorov, A. A.; Emelianchik, I.; Griesmayer, E.; Mechinsky, V.; Nargelas, S.; Sidletskiy, O.; Tamulaitis, G.; Tikhomirov, S. N.; Vaitkevicius, A.
2016-01-01
The time resolution of the detectors currently in use is limited by 50-70 ps due to the spontaneous processes involved in the development of the response signal, which forms after the relaxation of carriers generated during the interaction. In this study, we investigate the feasibility of exploiting sub-picosecond phenomena occurring after the interaction of scintillator material with ionizing radiation by probing the material with ultra-short laser pulses. One of the phenomena is the elastic polarization due to the local lattice distortion caused by the displacement of electrons and holes generated by ionization. The key feature of the elastic polarization is its short response time, which makes it prospective for using as an optically detectable time mark. The nonlinear optical absorption of femtosecond light pulses of appropriate wavelength is demonstrated to be a prospective tool to form the mark. This study was aimed at searching for inorganic crystalline media combining scintillation properties and non-...
Optical tsunamis: shoaling of shallow water rogue waves in nonlinear fibers with normal dispersion
International Nuclear Information System (INIS)
Wabnitz, Stefan
2013-01-01
In analogy with ocean waves running up towards the beach, shoaling of pre-chirped optical pulses may occur in the normal group-velocity dispersion regime of optical fibers. We present exact Riemann wave solutions of the optical shallow water equations and show that they agree remarkably well with the numerical solutions of the nonlinear Schrödinger equation, at least up to the point where a vertical pulse front develops. We also reveal that extreme wave events or optical tsunamis may be generated in dispersion tapered fibers in the presence of higher-order dispersion. (paper)
Directory of Open Access Journals (Sweden)
Kevin Schires
2011-09-01
Full Text Available We present the first comprehensive experimental study, to our knowledge, of the routes between nonlinear dynamics induced in a semiconductor laser under external optical injection based on an analysis of time-averaged measurements of the optical and RF spectra and phasors of real-time series of the laser output. The different means of analysis are compared for several types of routes and the benefits of each are discussed in terms of the identification and mapping of the nonlinear dynamics. Finally, the results are presented in a novel audio/video format that describes the evolution of the dynamics with the injection parameters.
Exact optical solitons in (n + 1)-dimensions with anti-cubic nonlinearity
Younis, Muhammad; Shahid, Iram; Anbreen, Sumaira; Rizvi, Syed Tahir Raza
2018-02-01
The paper studies the propagation of optical solitons in (n + 1)-dimensions under anti-cubic law of nonlinearity. The bright, dark and singular optical solitons are extracted using the extended trial equation method. The constraint conditions, for the existence of these solitons, are also listed. Additionally, a couple of other solutions known as singular periodic and Jacobi elliptic solutions, fall out as a by-product of this scheme. The obtained results are new and reported first time in (n + 1)-dimensions with anti-cubic law of nonlinearity.
Web Platform for Sharing Modeling Software in the Field of Nonlinear Optics
Dubenskaya, Julia; Kryukov, Alexander; Demichev, Andrey
2018-02-01
We describe the prototype of a Web platform intended for sharing software programs for computer modeling in the rapidly developing field of the nonlinear optics phenomena. The suggested platform is built on the top of the HUBZero open-source middleware. In addition to the basic HUBZero installation we added to our platform the capability to run Docker containers via an external application server and to send calculation programs to those containers for execution. The presented web platform provides a wide range of features and might be of benefit to nonlinear optics researchers.
Mapping the nonlinear optical susceptibility by noncollinear second-harmonic generation.
Larciprete, M C; Bovino, F A; Giardina, M; Belardini, A; Centini, M; Sibilia, C; Bertolotti, M; Passaseo, A; Tasco, V
2009-07-15
We present a method, based on noncollinear second-harmonic generation, to evaluate the nonzero elements of the nonlinear optical susceptibility. At a fixed incidence angle, the generated signal is investigated by varying the polarization state of both fundamental beams. The resulting polarization charts allows us to verify if Kleinman's symmetry rules can be applied to a given material or to retrieve the absolute value of the nonlinear optical tensor terms, from a reference measurement. Experimental measurements obtained from gallium nitride layers are reported. The proposed method does not require an angular scan and thus is useful when the generated signal is strongly affected by sample rotation.
Web Platform for Sharing Modeling Software in the Field of Nonlinear Optics
Directory of Open Access Journals (Sweden)
Dubenskaya Julia
2018-01-01
Full Text Available We describe the prototype of a Web platform intended for sharing software programs for computer modeling in the rapidly developing field of the nonlinear optics phenomena. The suggested platform is built on the top of the HUBZero open-source middleware. In addition to the basic HUBZero installation we added to our platform the capability to run Docker containers via an external application server and to send calculation programs to those containers for execution. The presented web platform provides a wide range of features and might be of benefit to nonlinear optics researchers.
International Nuclear Information System (INIS)
Bartlett, Stephen D.; Sanders, Barry C.
2002-01-01
Although universal continuous-variable quantum computation cannot be achieved via linear optics (including squeezing), homodyne detection, and feed-forward, inclusion of ideal photon-counting measurements overcomes this obstacle. These measurements are sometimes described by arrays of beam splitters to distribute the photons across several modes. We show that such a scheme cannot be used to implement ideal photon counting and that such measurements necessarily involve nonlinear evolution. However, this requirement of nonlinearity can be moved ''off-line,'' thereby permitting universal continuous-variable quantum computation with linear optics
Nonlinear optics and solid-state lasers advanced concepts, tuning-fundamentals and applications
Yao, Jianquan
2012-01-01
This book covers the complete spectrum of nonlinear optics and all solid state lasers.The book integrates theory, calculations and practical design, technology, experimental schemes and applications. With the expansion and further development of Laser technology, the wavelength spectrum of Lasers had to be enlarged, even to be tunable which requires the use of nonlinear optical and Laser tunable technology. It systematically summarizes and integrates the analysis of international achievements within the last 20 years in this field. It will be helpful for university teachers, graduate students as well as engineers.
International Nuclear Information System (INIS)
Makarov, V.A.
2004-01-01
The aim of the report is to describe the history of the Moscow University Coherent and Nonlinear Optics School headed by R.V. Khokhlov and S.A. Akhmanov being a part of the history of the Russian efforts to investigate into quantum electronics. The reports describes briefly the most significant results of the mentioned School activity, in particular, thermonuclear reactions initiated by laser pulses in plasma; the procedure to accelerate electrons up to 1 GeV using the present-day lasers; the nonlinear-optical analogues of the Faraday and the Kerr effects [ru
Structural, Linear, and Nonlinear Optical and Mechanical Properties of New Organic L-Serine Crystal
Directory of Open Access Journals (Sweden)
K. Rajesh
2014-01-01
Full Text Available Nonlinear optical single crystal of organic amino acid L-Serine (LS was grown by slow evaporation technique. Solubility study of the compound was measured and metastable zone width was found. Single crystal X-ray diffraction study was carried out for the grown crystal. The linear and nonlinear optical properties of the crystal were confirmed by UV-Vis analysis and powder SHG tester. FT-IR spectrum was recorded and functional groups were analyzed. Vickers’ microhardness studies showed the mechanical strength of the grown crystal. Laser damage threshold value of the crystal was calculated. Photoconductivity studies reveal the conductivity of the crystal.
TITLE PAGE Linear and nonlinear optical properties of 4 ...
Indian Academy of Sciences (India)
57
optical effects viz. reverse saturable absorption and self-defocusing of laser beam. ... Defect Analysis, Mechanical stability, UV-visible spectroscopy, Refractive index .... for geometry optimization in gas phase and in the solvent phase (ethanol).
Growth and characterization of nonlinear optical single crystals: bis ...
Indian Academy of Sciences (India)
Administrator
molecules have received great attention for NLO applica- tions. However ... Figure 3. Single crystals of bis(cyclohexylammonium) terephthalate (crystal a) and cyclohexylammo- .... from ground state to higher energy states.17 Optical window ...
Linear and nonlinear optical susceptibilities in a laterally coupled quantum-dot–quantum-ring system
International Nuclear Information System (INIS)
Zeng, Zaiping; Garoufalis, Christos S.; Baskoutas, Sotirios
2014-01-01
Linear and nonlinear optical susceptibilities in a laterally coupled quantum-dot–quantum-ring system have been theoretically studied. In general, we find that the structure parameters of the coupled system significantly affect the optical susceptibilities. The enhancement of the coupling effects between the dot and ring is found to increase considerably the optical susceptibilities and redshift drastically the transition energies. Comparing to the linear susceptibility, the nonlinear optical susceptibility is found to be more sensitive to the variation of the structure parameters. A comprehensive analysis of the electron probability density movement with respect to the modification of the structure parameters is provided, which offers a unique perspective of the ground-state localization. - Highlights: • Optical susceptibilities in a quantum-dot–quantum-ring system are studied. • The structure parameters significantly affect the optical susceptibilities. • The enhancement of the coupling effects increases the optical susceptibilities. • The nonlinear susceptibility is more sensitive to the change in structure parameters. • A comprehensive analysis of the electron probability density movement is provided
Oscillations in the interactions among multiple solitons in an optical fibre
Energy Technology Data Exchange (ETDEWEB)
Hu, Wen-Qiang; Gao, Yi-Tian; Zhao, Chen; Feng, Yu-Jie; Su, Chuan-Qi [Beijing University of Aeronautics and Astronautics (China). Ministry of Education Key Laboratory of Fluid Mechanics; Beijing University of Aeronautics and Astronautics (China). National Laboratory for Computational Fluid Dynamics
2016-07-01
In this article, under the investigation on the interactions among multiple solitons for an eighth-order nonlinear Schroedinger equation in an optical fibre, oscillations in the interaction zones are observed theoretically. With different coefficients of the operators in this equation, we find that (1) the oscillations in the solitonic interaction zones have different forms with different spectral parameters of this equation; (2) the oscillations in the interactions among the multiple solitons are affected by the choice of spectral parameters, the dispersive effects and nonlinearity of the eighth-order operator; (3) the second-, fifth-, sixth-, and seventh-order operators restrain oscillations in the solitonic interaction zones and the higher-order operators have stronger attenuated effects than the lower ones, while the third- and fourth-order operators stimulate and extend the scope of oscillations.
Nonlinear optical effects from Au nanoparticles prepared by laser plasmas in water
Energy Technology Data Exchange (ETDEWEB)
Fazio, E., E-mail: enfazio@unime.it [Dipartimento di Fisica della Materia e Ingegneria Elettronica, Universitá di Messina, V.le F. Stagno d’Alcontres 31, I-98166, Messina (Italy); Neri, F. [Dipartimento di Fisica della Materia e Ingegneria Elettronica, Universitá di Messina, V.le F. Stagno d’Alcontres 31, I-98166, Messina (Italy)
2013-05-01
The optical limiting properties of Au nanoparticles prepared by laser generated plasmas in water were investigated. The ablation processes were carried out irradiating an Au target with the second harmonic (532 nm) output of a Nd:YAG laser, changing the water level above the target, the lens position and the laser pulse energy. Different surface morphologies, from isolated nearly spherical nanoparticles to elongated structures, were observed by TEM imaging. A significant nonlinear optical response was probed by the Z-scan technique. The efficiency and the nature of the nonlinear response are found to be strongly dependent on the morphological properties of the nanostructures. The third order optical susceptibility χ{sup (3)} assumes the values of 1.83 × 10{sup −6} esu and 6.34 × 10{sup −6} esu for the smaller nanoparticles size obtained at the lower ablation energies (10–20 mJ), 8.25 × 10{sup −6} esu and 2.13 × 10{sup −5} esu for the particles agglomerations obtained at the higher ablation energies (50–100 mJ). The high value of χ{sup (3)} and the possibility to tailor the nonlinear optical response by changing the morphological properties of the Au nanostructures make them interesting materials for potential applications in the nonlinear optics field.
Garbovskiy, Y.; Klimusheva, G.; Mirnaya, T.
2016-09-01
Mesomorphic metal alkanoates is very promising yet overlooked class of nonlinear-optical materials. Metal alkanoates can exhibit a broad variety of condensed states of matter including solid crystals, plastic crystals, lyotropic and thermotropic ionic liquid crystals, liquids, mesomorphic glasses, and Langmuir-Blodgett films. Glass-forming properties of metal alkanoates combined with their use as nano-reactors and anisotropic host open up simple and efficient way to design various photonic nanomaterials. Despite very interesting physics, the experimental data on optical and nonlinearoptical properties of such materials are scarce. The goal of the present paper is to fill the gap by discussing recent advances in the field of photonic materials made of metal alkanoates, organic dyes, and nanoparticles. Optical and nonlinear-optical properties of the following materials are reviewed: (i) mesomorphic glass doped with organic dyes; (ii) smectic glass composed of cobalt alkanoates; (iii) semiconductor nanoparticles embedded in a glassy host; (iv) metal nanoparticles - glass (the cobalt octanoate) nanocomposites.
Nonlinear optical properties of poly(methyl methacrylate) thin films doped with Bixa Orellana dye
Energy Technology Data Exchange (ETDEWEB)
Zongo, S., E-mail: sidiki@tlabs.ac.za [UNESCO-UNISA Africa Chair in Nanosciences/Nanotechnology, College of Graduate Studies, University of South Africa, Muckleneuk ridge, POBox 392, Pretoria (South Africa); Nanosciences African Network (NANOAFNET), iThemba LABS-National Research Foundation, 1 OldFaure road, Somerset West 7129, POBox 722, Somerset West, Western Cape Province (South Africa); Kerasidou, A.P. [LUNAM Université, Université d’Angers, CNRS UMR 6200, Laboratoire MOLTECH-Anjou, 2 Bd Lavoisier, 49045 Angers Cedex (France); Sone, B.T.; Diallo, A. [UNESCO-UNISA Africa Chair in Nanosciences/Nanotechnology, College of Graduate Studies, University of South Africa, Muckleneuk ridge, POBox 392, Pretoria (South Africa); Nanosciences African Network (NANOAFNET), iThemba LABS-National Research Foundation, 1 OldFaure road, Somerset West 7129, POBox 722, Somerset West, Western Cape Province (South Africa); Mthunzi, P. [Council for Scientific and Industrial Research, P O Box 395, Pretoria 0001 (South Africa); Iliopoulos, K. [LUNAM Université, Université d’Angers, CNRS UMR 6200, Laboratoire MOLTECH-Anjou, 2 Bd Lavoisier, 49045 Angers Cedex (France); Institute of Chemical Engineering Sciences, Foundation for Research and Technology Hellas (FORTH/ICE-HT), 26504 Patras (Greece); Nkosi, M. [Nanosciences African Network (NANOAFNET), iThemba LABS-National Research Foundation, 1 OldFaure road, Somerset West 7129, POBox 722, Somerset West, Western Cape Province (South Africa); and others
2015-06-15
Highlights: • We studied the linear and nonlinear optical properties of hybrid Bixa Orellana dye doped PMMA thin film. • We investigated the linear optical properties by means of UV/Vis, FTIR and Fluorescence. • We used Tauc - Lorentz model to evaluate linear optical parameters (n &k) with relative maximum of 1.456 at 508.5, 523.79 and 511.9 nm for n is observed while the maximum of k varies from 0.070 to 0.080. • We evaluated nonlinear third order susceptibility which was found to be 1.00 × 10{sup −21} m{sup 2} V{sup −2} or 0.72 × 10{sup −13} esu. - Abstract: Natural dyes with highly delocalized π-electron systems are considered as promising organic materials for nonlinear optical applications. Among these dyes, Bixa Orellana dye with extended π-electron delocalization is one of the most attractive dyes. Bixa Orellana dye-doped Poly(methyl methacrylate) (PMMA) thin films were prepared through spin coating process for linear and nonlinear optical properties investigation. Atomic force microscopy (AFM) was used to evaluate the roughness of the thin films. The optical constants n and k were evaluated by ellipsometric spectroscopy. The refractive index had a maximum of about 1.456 at 508.5, 523.79 and 511.9 nm, while the maximum of k varies from 0.070 to 0.080 with the thickness. The third order nonlinear optical properties of the hybrid Bixa Orellana dye-PMMA polymer were investigated under 30 ps laser irradiation at 1064 nm with a repetition rate of 10 Hz. In particular the third-order nonlinear susceptibility has been determined by means of the Maker Fringes technique. The nonlinear third order susceptibility was found to be 1.00 × 10{sup −21} m{sup 2} V{sup −2} or 0.72 × 10{sup −13} esu. Our studies provide concrete evidence that the hybrid-PMMA composites of Bixa dye are prospective candidates for nonlinear material applications.
Measurement of rotational dynamics by the simultaneous nonlinear analysis of optical and EPR data.
Hustedt, E J; Cobb, C E; Beth, A H; Beechem, J M
1993-01-01
In the preceding companion article in this issue, an optical dye and a nitroxide radical were combined in a new dual function probe, 5-SLE. In this report, it is demonstrated that time-resolved optical anisotropy and electron paramagnetic resonance (EPR) data can be combined in a single analysis to measure rotational dynamics. Rigid-limit and rotational diffusion models for simulating nitroxide EPR data have been incorporated into a general non-linear least-squares procedure based on the Marq...
Cross-talk dynamics of optical solitons in a broadband Kerr nonlinear system with weak cubic loss
International Nuclear Information System (INIS)
Peleg, Avner; Nguyen, Quan M.; Chung, Yeojin
2010-01-01
We study the dynamics of fast soliton collisions in a Kerr nonlinear optical waveguide with weak cubic loss. We obtain analytic expressions for the amplitude and frequency shifts in a single two-soliton collision and show that the impact of a fast three-soliton collision is given by the sum of the two-soliton interactions. Our analytic predictions are confirmed by numerical simulations with the perturbed nonlinear Schroedinger (NLS) equation. Furthermore, we show that the deterministic collision-induced dynamics of soliton amplitudes in a broadband waveguide system with N frequency channels is described by a Lotka-Volterra model for N competing species. For a two-channel system we find that stable transmission with equal prescribed amplitudes can be achieved by a proper choice of linear amplifier gain. The predictions of the Lotka-Volterra model are confirmed by numerical solution of a perturbed coupled-NLS model.
Second order optical nonlinearity in silicon by symmetry breaking
Energy Technology Data Exchange (ETDEWEB)
Cazzanelli, Massimo, E-mail: massimo.cazzanelli@unitn.it [Laboratorio IdEA, Dipartimento di Fisica, Università di Trento, via Sommarive, 14 Povo (Trento) (Italy); Schilling, Joerg, E-mail: joerg.schilling@physik.uni-halle.de [Centre for Innovation Competence SiLi-nano, Martin-Luther-University Halle-Wittenberg, Karl-Freiherr-von-Fritsch Str. 3, 06120 Halle (Germany)
2016-03-15
Although silicon does not possess a dipolar bulk second order nonlinear susceptibility due to its centro-symmetric crystal structure, in recent years several attempts were undertaken to create such a property in silicon. This review presents the different sources of a second order susceptibility (χ{sup (2)}) in silicon and the connected second order nonlinear effects which were investigated up to now. After an introduction, a theoretical overview discusses the second order nonlinearity in general and distinguishes between the dipolar contribution—which is usually dominating in non-centrosymmetric structures—and the quadrupolar contribution, which even exists in centro-symmetric materials. Afterwards, the classic work on second harmonic generation from silicon surfaces in reflection measurements is reviewed. Due to the abrupt symmetry breaking at surfaces and interfaces locally a dipolar second order susceptibility appears, resulting in, e.g., second harmonic generation. Since the bulk contribution is usually small, the study of this second harmonic signal allows a sensitive observation of the surface/interface conditions. The impact of covering films, strain, electric fields, and defect states at the interfaces was already investigated in this way. With the advent of silicon photonics and the search for ever faster electrooptic modulators, the interest turned to the creation of a dipolar bulk χ{sup (2)} in silicon. These efforts have been focussing on several experiments applying an inhomogeneous strain to the silicon lattice to break its centro-symmetry. Recent results suggesting the impact of electric fields which are exerted from fixed charges in adjacent covering layers are also included. After a subsequent summary on “competing” concepts using not Si but Si-related materials, the paper will end with some final conclusions, suggesting possible future research direction in this dynamically developing field.
Beam-Based Nonlinear Optics Corrections in Colliders
Pilat, Fulvia Caterina; Malitsky, Nikolay; Ptitsyn, Vadim
2005-01-01
A method has been developed to measure and correct operationally the non-linear effects of the final focusing magnets in colliders, which gives access to the effects of multi-pole errors by applying closed orbit bumps, and analyzing the resulting tune and orbit shifts. This technique has been tested and used during 3 years of RHIC (the Relativistic Heavy Ion Collider at BNL) operations. I will discuss here the theoretical basis of the method, the experimental set-up, the correction results, the present understanding of the machine model, the potential and limitations of the method itself as compared with other non linear correction techniques.
Real-Time Implementation of Nonlinear Optical Processing Functions.
1986-09-30
information capacity) with the nonlinear error correction properties of associative neural nets such as the Hopfield model. Analogies between holography...symnolic ma.Ip’:ation Th.e error correcting -apart" :ty of non" ;n-ar associative merTtnies is necessary for s’uch structu-res Experimerta. results... geometrica snapes in contact ’A,.n a c-:’:ser ’Figure 51a’ ., and a spher:cal 4:verg.ng reference -eam Upion :"um’latlon of t -" c-’gram by the object beam
Single-pulse CARS based multimodal nonlinear optical microscope for bioimaging.
Kumar, Sunil; Kamali, Tschackad; Levitte, Jonathan M; Katz, Ori; Hermann, Boris; Werkmeister, Rene; Považay, Boris; Drexler, Wolfgang; Unterhuber, Angelika; Silberberg, Yaron
2015-05-18
Noninvasive label-free imaging of biological systems raises demand not only for high-speed three-dimensional prescreening of morphology over a wide-field of view but also it seeks to extract the microscopic functional and molecular details within. Capitalizing on the unique advantages brought out by different nonlinear optical effects, a multimodal nonlinear optical microscope can be a powerful tool for bioimaging. Bringing together the intensity-dependent contrast mechanisms via second harmonic generation, third harmonic generation and four-wave mixing for structural-sensitive imaging, and single-beam/single-pulse coherent anti-Stokes Raman scattering technique for chemical sensitive imaging in the finger-print region, we have developed a simple and nearly alignment-free multimodal nonlinear optical microscope that is based on a single wide-band Ti:Sapphire femtosecond pulse laser source. Successful imaging tests have been realized on two exemplary biological samples, a canine femur bone and collagen fibrils harvested from a rat tail. Since the ultra-broad band-width femtosecond laser is a suitable source for performing high-resolution optical coherence tomography, a wide-field optical coherence tomography arm can be easily incorporated into the presented multimodal microscope making it a versatile optical imaging tool for noninvasive label-free bioimaging.
International Nuclear Information System (INIS)
Ghosh, Binita; Chakraborty, Purushottam
2011-01-01
Silver ion implantations in fused silica glasses have been made to synthesize silver nanocluster-glass composites and a combination of 'Anti-Resonant Interferometric Nonlinear Spectroscopy (ARINS)' and 'Z-scan' techniques has been employed for the measurement of the third-order optical susceptibility of these nanocomposites. The ARINS technique utilizes the dressing of two unequal-intensity counter-propagating pulsed optical beams with differential nonlinear phases, which occurs upon traversing the sample. This difference in phase manifests itself in the intensity-dependent transmission, measurement of which enables us to extract the values of nonlinear refractive index (η 2 ) and nonlinear absorption coefficient (β), finally yielding the real and imaginary parts of the third-order dielectric susceptibility (χ (3) ). The real and imaginary parts of χ (3) are obtained in the orders of 10 -10 e.s.u for silver nanocluster-glass composites. The present value of χ (3) , to our knowledge, is extremely accurate and much more reliable compared to the values previously obtained by other workers for similar silver-glass nanocomposites using only Z-scan technique. Optical nonlinearity has been explained to be due to two-photon absorption in the present nanocomposite glasses and is essentially of electronic origin.
THEORETICAL EVALUATION OF NONLINEAR EFFECTS ON OPTICAL WDM NETWORKS WITH VARIOUS FIBER TYPES
Directory of Open Access Journals (Sweden)
YASIN M. KARFAA
2010-09-01
Full Text Available A theoretical study is carried out to evaluate the performance of an opticalwavelength division multiplexing (WDM network transmission system in the presenceof crosstalk due to optical fiber nonlinearities. The most significant nonlinear effects inthe optical fiber which are Cross-Phase Modulation (XPM, Four-Wave Mixing (FWM,and Stimulated Raman Scattering (SRS are investigated. Four types of optical fiber areincluded in the analysis; these are: single-mode fiber (SMF, dispersion compensationfiber (DCF, non-zero dispersion fiber (NZDF, and non-zero dispersion shifted fiber(NZDSF. The results represent the standard deviation of nonlinearity induced crosstalknoise power due to FWM and SRS, XPM power penalty for SMF, DCF, NZDF, andNZDSF types of fiber, besides the Bit Error Rate (BER for the three nonlinear effectsusing standard fiber type (SMF. It is concluded that three significant fiber nonlinearitiesare making huge limitations against increasing the launched power which is desired,otherwise, lower values of launched power limit network expansion including length,distance, covered areas, and number of users accessing the WDM network, unlesssuitable precautions are taken to neutralize the nonlinear effects. Besides, various fibertypes are not behaving similarly towards network parameters.
Nonlinear Optical Response of Polar Semiconductors in the Terahertz Range
Roman, Eric; Yates, Jonathan; Veithen, Marek; Vanderbilt, David; Souza, Ivo
2006-03-01
Using the Berry-phase finite-field method, we compute from first-principles the recently measured infrared (IR) dispersion of the nonlinear susceptibility (2)circ in III-V zincblende semiconductors. At far-IR (terahertz) frequencies, in addition to the purely electronic response (2)circ∞, the total (2)circ depends on three other parameters, C1, C2, and C3, describing the contributions from ionic motion. They relate to the TO Raman polarizability and the second-order displacement-induced dielectric polarization and forces, respectively. Contrary to a widely-accepted model, but in agreement with the recent experiments on GaAs, ^1 we find that the contribution from mechanical anharmonicity dominates over electrical anharmonicity. By using Richardson extrapolation to evaluate the Berry's phase in k-space by finite differences, we are able to improve the convergence of the nonlinear susceptibility from the usual O[(δk)^2] to O[(δk)^4], dramatically reducing the computational cost. T. Dekorsy, V. A. Yakovlev, W. Seidel, M. Helm, and F. Keilmann, Phys. Rev. Lett. 90, 055508 (2003). C. Flytzanis, Phys. Rev. B 6, 1264 (1972). R. Umari and A. Pasquarello, Phys. Rev. B 68, 085114 (2003).
Towards modeling of nonlinear laser-plasma interactions with hydrocodes: The thick-ray approach
Colaïtis, A.; Duchateau, G.; Nicolaï, P.; Tikhonchuk, V.
2014-03-01
This paper deals with the computation of laser beam intensity in large-scale radiative hydrocodes applied to the modeling of nonlinear laser-plasma interactions (LPIs) in inertial confinement fusion (ICF). The paraxial complex geometrical optics (PCGO) is adapted for light waves in an inhomogeneous medium and modified to include the inverse bremsstrahlung absorption and the ponderomotive force. This thick-ray model is compared to the standard ray-tracing (RT) approach, both in the chic code. The PCGO model leads to different power deposition patterns and better diffraction modeling compared to standard RT codes. The intensity-reconstruction technique used in RT codes to model nonlinear LPI leads to artificial filamentation and fails to reproduce realistic ponderomotive self-focusing distances, intensity amplifications, and density channel depletions, whereas PCGO succeeds. Bundles of Gaussian thick rays can be used to model realistic non-Gaussian ICF beams. The PCGO approach is expected to improve the accuracy of ICF simulations and serve as a basis to implement diverse LPI effects in large-scale hydrocodes.
Vijayalakshmi, A.; Vidyavathy, B.; Vinitha, G.
2016-08-01
Isonicotinamide p-nitrophenol (ICPNP), a new organic material, was synthesized using methanol solvent. Single crystals of ICPNP were grown using a slow evaporation solution growth technique. Crystal structure of ICPNP is elucidated by single crystal X-ray diffraction analysis. It belongs to monoclinic crystal system with space group of P21/c. It forms two dimensional networks by O-H…O, N-H…O and C-H…O hydrogen bonds. The molecular structure of ICPNP was further confirmed by Fourier transform infrared (FTIR) spectral analysis. The optical transmittance range and the lower cut-off wavelength (421 nm) with the optical band gap (2.90 eV) of the ICPNP crystal were determined by UV-vis-NIR spectral study. Thermal behavior of ICPNP was studied by thermo gravimetric and differential thermal analyses (TG/DTA). The relative dielectric permittivity was calculated for various temperature ranges. Laser damage threshold of ICPNP crystal was found to be 1.9 GW/cm2 using an Nd:YAG laser. A Z-scan technique was employed to measure the nonlinear absorption coefficient, nonlinear refractive index and nonlinear optical susceptibility. Optical limiting behavior of ICPNP was observed at 35 mW input power.
Non-linear optical studies of adsorbates: Spectroscopy and dynamics
International Nuclear Information System (INIS)
Zhu, Xiangdong.
1989-08-01
In the first part of this thesis, we have established a systematic procedure to apply the surface optical second-harmonic generation (SHG) technique to study surface dynamics of adsorbates. In particular, we have developed a novel technique for studies of molecular surface diffusions. In this technique, the laser-induced desorption with two interfering laser beams is used to produce a monolayer grating of adsorbates. The monolayer grating is detected with diffractions of optical SHG. By monitoring the first-order second-harmonic diffraction, we can follow the time evolution of the grating modulation from which we are able to deduce the diffusion constant of the adsorbates on the surface. We have successfully applied this technique to investigate the surface diffusion of CO on Ni(111). The unique advantages of this novel technique will enable us to readily study anisotropy of a surface diffusion with variable grating orientation, and to investigate diffusion processes of a large dynamic range with variable grating spacings. In the second part of this work, we demonstrate that optical infrared-visible sum-frequency generation (SFG) from surfaces can be used as a viable surface vibrational spectroscopic technique. We have successfully recorded the first vibrational spectrum of a monolayer of adsorbates using optical infrared-visible SFG. The qualitative and quantitative correlation of optical SFG with infrared absorption and Raman scattering spectroscopies are examined and experimentally demonstrated. We have further investigated the possibility to use transient infrared-visible SFG to probe vibrational transients and ultrafast relaxations on surfaces. 146 refs
Non-linear optical studies of adsorbates: Spectroscopy and dynamics
Energy Technology Data Exchange (ETDEWEB)
Zhu, Xiangdong.
1989-08-01
In the first part of this thesis, we have established a systematic procedure to apply the surface optical second-harmonic generation (SHG) technique to study surface dynamics of adsorbates. In particular, we have developed a novel technique for studies of molecular surface diffusions. In this technique, the laser-induced desorption with two interfering laser beams is used to produce a monolayer grating of adsorbates. The monolayer grating is detected with diffractions of optical SHG. By monitoring the first-order second-harmonic diffraction, we can follow the time evolution of the grating modulation from which we are able to deduce the diffusion constant of the adsorbates on the surface. We have successfully applied this technique to investigate the surface diffusion of CO on Ni(111). The unique advantages of this novel technique will enable us to readily study anisotropy of a surface diffusion with variable grating orientation, and to investigate diffusion processes of a large dynamic range with variable grating spacings. In the second part of this work, we demonstrate that optical infrared-visible sum-frequency generation (SFG) from surfaces can be used as a viable surface vibrational spectroscopic technique. We have successfully recorded the first vibrational spectrum of a monolayer of adsorbates using optical infrared-visible SFG. The qualitative and quantitative correlation of optical SFG with infrared absorption and Raman scattering spectroscopies are examined and experimentally demonstrated. We have further investigated the possibility to use transient infrared-visible SFG to probe vibrational transients and ultrafast relaxations on surfaces. 146 refs.
Local-field enhancement effect on the nonlinear optical response of gold-silver nanoplanets.
Cesca, T; Calvelli, P; Battaglin, G; Mazzoldi, P; Mattei, G
2012-02-13
We report on the nonlinear optical properties of Au-Ag nanoplanets produced by ion implantation and irradiation in silica, experimentally investigated by means of the single beam z-scan technique. The measurements provided experimental evidence of the intense local-field enhancement effect theoretically demonstrated for these plasmonic nanosystems. In particular, this has a dramatic impact on their nonlinear absorption behavior and results in a tunable changeover from reverse saturable absorption to saturable absorption by slightly varying the pump intensity and in the possibility to activate and observe nonlinear phenomena of the electron dynamics otherwise unaccessible in the intensity range that can be employed to study these materials. Finally, for the nanoplanet configuration we found a dramatic decrease of the intensity-dependent absorption coefficient, which could be very promising for obtaining optical gain materials.
International Nuclear Information System (INIS)
Tomita, Yasuo; Matsushima, Shun-suke; Yamagami, Ryu-ichi; Jinzenji, Taka-aki; Sakuma, Shohei; Liu, Xiangming; Izuishi, Takuya; Shen, Qing
2017-01-01
We describe the nonlinear optical properties of inorganic-organic nanocomposite films in which semiconductor CdSe quantum dots as high as 6.8 vol.% are dispersed. Open/closed Z-scan measurements, degenerate multi-wave mixing and femtosecond pump-probe/transient grating measurements are conducted. It is shown that the observed fifth-order optical nonlinearity has the cascaded third-order contribution that becomes prominent at high concentrations of CdSe QDs. It is also shown that there are picosecond-scale intensity-dependent and nanosecond-scale intensity-independent decay components in absorptive and refractive nonlinearities. The former is caused by the Auger process, while the latter comes from the electron-hole recombination process. (paper)
Energy Technology Data Exchange (ETDEWEB)
Castro, Hemerson P. S.; Alencar, Márcio A. R. C.; Hickmann, Jandir M. [Optics and Materials Group–OPTMA, Universidade Federal de Alagoas, CAIXA POSTAL 2051, 57061-970 Maceió (Brazil); Wender, Heberton [Brazilian Synchrotron National Laboratory (LNLS), CNPEM, Rua Giuseppe Máximo Scolfaro 10.000, 13083-970 Campinas (Brazil); Department of Physics, Universidade Federal do Mato Grosso do Sul, 79070-900, Campo Grande (Brazil); Teixeira, Sergio R. [Institute of Physics, Universidade Federal do Rio Grande do Sul, 91501-970, Porto Alegre (Brazil); Dupont, Jairton [Laboratory of Molecular Catalysis, Institute of Chemistry, Universidade Federal do Rio Grande do Sul, 91501-970, Porto Alegre (Brazil)
2013-11-14
The nonlinear optical responses of gold nanoparticles dispersed in castor oil produced by sputtering deposition were investigated, using the thermally managed Z-scan technique. Particles with spherical shape and 2.6 nm of average diameter were obtained and characterized by transmission electron microscopy and small angle X-ray scattering. This colloid was highly stable, without the presence of chemical impurities, neither stabilizers. It was observed that this system presents a large refractive third-order nonlinear response and a negligible nonlinear absorption. Moreover, the evaluation of the all-optical switching figures of merit demonstrated that the colloidal nanoparticles prepared by sputtering deposition have a good potential for the development of ultrafast photonic devices.
Nonlinear optical properties of poly(methyl methacrylate) thin films doped with Bixa Orellana dye
CSIR Research Space (South Africa)
Zongo, S
2015-06-01
Full Text Available Natural dyes with highly delocalized p-electron systems are considered as promising organic materials for nonlinear optical applications. Among these dyes, Bixa Orellana dye with extended p-electron delocalization is one of the most attractive dyes...
Guanylurea(1+) hydrogen phosphite: study of linear and nonlinear optical properties
Czech Academy of Sciences Publication Activity Database
Fridrichová, M.; Kroupa, Jan; Němec, I.; Císařová, I.; Chvostová, Dagmar
2010-01-01
Roč. 83, 10-11 (2010), s. 761-767 ISSN 0141-1594 R&D Projects: GA ČR GA203/09/0878 Institutional research plan: CEZ:AV0Z10100520 Keywords : non-centrosymmetric * guanylurea * refractive indices * nonlinear optics Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.006, year: 2010
All-optical switching in lithium niobate directional couplers with cascaded nonlinearity
Schiek, R.; Baek, Y.; Krijnen, Gijsbertus J.M.; Stegeman, G.I.; Baumann, I.; Sohler, W.
1996-01-01
We report on intensity-dependent switching in lithium niobate directional couplers. Large nonlinear phase shifts that are due to cascading detune the coupling between the coupler branches, which makes all-optical switching possible. Depending on the input intensity, the output could be switched
Nonlinear Optical Functions in Crystalline and Amorphous Silicon-on-Insulator Nanowires
DEFF Research Database (Denmark)
Baets, R.; Kuyken, B.; Liu, X.
2012-01-01
Silicon-on-Insulator nanowires provide an excellent platform for nonlinear optical functions in spite of the two-photon absorption at telecom wavelengths. Work on both crystalline and amorphous silicon nanowires is reviewed, in the wavelength range of 1.5 to 2.5 µm....
International Nuclear Information System (INIS)
Fernández-Hernández, Roberto Carlos; Gleason-Villagran, Roberto; Rodríguez-Fernández, Luis; Crespo-Sosa, Alejandro; Cheang-Wong, Juan Carlos; López-Suárez, Alejandra; Oliver, Alicia; Reyes-Esqueda, Jorge Alejandro; Torres-Torres, Carlos; Rangel-Rojo, Raúl
2012-01-01
Au and Ag isotropic and anisotropic nanocomposites were prepared using the ion implantation technique. Their optical properties were studied at several wavelengths in the optical range 300–800 nm, across their plasmon resonances. The linear regime was characterized by measuring the absorption spectrum and the third-order nonlinear regime by means of the Z-scan technique using a tunable picosecond pulsed laser system (26 ps). Open-aperture Z-scan traces show a superposition of different optical nonlinear absorption (NLA) processes in the whole range studied. We associate these phenomena with the excitation of inter- and intra-band electronic transitions, which contribute with a positive sign to NLA, and to the formation of hot-electrons, which contribute with opposite sign to NLA. Closed-aperture traces for measuring nonlinear refraction (NLR) show different signs for Au and Ag samples, and a change of sign in Au is found when purely inter-band transitions are excited. In this work, for the appropriate wavelength, it is worth remarking on the free-electron response to the exciting light and its strong contribution to the nonlinear optical properties for low (intra-band) and high (hot-electrons) irradiances. (paper)
Knoester, Jasper; Mukamel, Shaul
1990-01-01
A general scheme is presented for calculating the nonlinear optical response in condensed phases that provides a unified picture of excitons, polaritons, retardation, and local-field effects in crystals and in disordered systems. A fully microscopic starting point is taken by considering the
Optical mixing of microwave signals in a nonlinear semiconductor laser amplifier modulator.
Capmany, José; Sales, Salvador; Pastor, Daniel; Ortega, Beatriz
2002-02-11
In this paper we propose and evaluate the optical mixing of RF signals by means of exploiting the nonlinearity of a SLA modulator. The results show the potential for devices with low conversion losses (and even gain) and polarization insensitivity and reduced insertion losses.
Li, Jin Hua; Xu, Hui; Sun, Ting Ting; Pei, Shi Xin; Ren, Hai Dong
2018-05-01
We analyze in detail the effects of the intermode nonlinearity (IEMN) and intramode nonlinearity (IRMN) on modulation instability (MI) in randomly birefringent two-mode optical fibers (RB-TMFs). In the anomalous dispersion regime, the MI gain enhances significantly as the IEMN and IRMN coefficients increases. In the normal dispersion regime, MI can be generated without the differential mode group delay (DMGD) effect, as long as the IEMN coefficient between two distinct modes is above a critical value, or the IRMN coefficient inside a mode is below a critical value. This critical IEMN (IRMN) coefficient depends strongly on the given IRMN (IEMN) coefficient and DMGD for a given nonlinear RB-TMF structure, and is independent on the input total power, the power ratio distribution and the group velocity dispersion (GVD) ratio between the two modes. On the other hand, in contrast to the MI band arising from the pure effect of DMGD in the normal dispersion regime, where MI vanishes after a critical total power, the generated MI band under the combined effects of IEMN and IRMN without DMGD exists for any total power and enhances with the total power. The MI analysis is verified numerically by launching perturbed continuous waves (CWs) with wave propagation method.
Maidur, Shivaraj R.; Jahagirdar, Jitendra R.; Patil, Parutagouda Shankaragouda; Chia, Tze Shyang; Quah, Ching Kheng
2018-01-01
We report synthesis, characterizations, structure-property relationships, and third-order nonlinear optical studies for two new chalcone derivatives, (2E)-1-(anthracen-9-yl)-3-(4-bromophenyl)prop-2-en-1-one (Br-ANC) and (2E)-1-(anthracen-9-yl)-3-(4-chlorophenyl)prop-2-en-1-one (Cl-ANC). These derivatives were crystallized in the centrosymmetric monoclinic P21/c crystal structure. The intermolecular interactions of both the crystals were visualized by Hirshfeld surface analyses (HSA). The crystals are thermally stable up to their melting points (180.82 and 191.16 °C for Cl-ANC and Br-ANC, respectively). The geometry optimizations, FT-IR spectra, 1H and 13C NMR spectra, electronic absorption spectra, electronic transitions, and HOMO-LUMO energy gaps were studied by Density Functional Theory (DFT) at B3LYP/6-311+G(d, p) level. The theoretical results provide excellent agreement with experimental findings. The electric dipole moments, static polarizabilities, molecular electrostatic potentials (MEP) and global chemical reactivity descriptors (GCRD) were also theoretically computed. The materials exhibited good nonlinear absorption (NLA), nonlinear refraction (NLR) and optical limiting (OL) behavior under diode-pumped solid-state (DPSS) continuous wave (CW) laser excitation (532 nm and 200 mW). The NLO parameters such as NLA coefficient (β∼10-5 cmW-1), NLR index (n2∼10-10 cm2 W-1) and third-order NLO susceptibilities (χ(3) ∼10-7 esu) were measured. Further, we estimated one-photon and two-photon figures of merit, which satisfy the demands (W > 1 and T < 1) for all-optical switching. Thus, the present chalcone derivatives with anthracene moiety are potential materials for OL and optical switching applications.
Nonlinear theory of surface-wave--particle interactions in a cylindrical plasma
International Nuclear Information System (INIS)
Dengra, A.; Palop, J.I.F.
1994-01-01
This work is an application of the specular reflection hypothesis to the study of the nonlinear surface-wave--particle interactions in a cylindrical plasma. The model is based on nonlinear resolution of the Vlasov equation by the method of characteristics. The expression obtained for the rate of increase of kinetic energy per electron has permitted us to investigate the temporal behavior of nonlinear collisionless damping for different situations as a function of the critical parameters
RCLED Optimization and Nonlinearity Compensation in a Polymer Optical Fiber DMT System
Directory of Open Access Journals (Sweden)
Pu Miao
2016-09-01
Full Text Available In polymer optical fiber (POF systems, the nonlinear transfer function of the resonant cavity light emitting diode (RCLED drastically degrades the communication performance. After investigating the characteristics of the RCLED nonlinear behavior, an improved digital look-up-table (LUT pre-distorter, based on an adaptive iterative algorithm, is proposed. Additionally, the system parameters, including the bias current, the average electrical power, the LUT size and the step factor are also jointly optimized to achieve a trade-off between the system linearity, reliability and the computational complexity. With the proposed methodology, both the operating point and efficiency of RCLED are enhanced. Moreover, in the practical 50 m POF communication system with the discrete multi-tone (DMT modulation, the bit error rate performance is improved by over 12 dB when RCLED is operating in the nonlinear region. Therefore, the proposed pre-distorter can both resist the nonlinearity and improve the operating point of RCLED.
Ultrafast nonlinear optical studies of equiaxed CuNbO3 microstructures
Priyadarshani, N.; Sabari Girisun, T. C.; Venugopal Rao, S.
2017-08-01
Diverse microstructures of monoclinic copper niobate (m-CuNbO3) were synthesized by solid-state reaction (900 °C, 3-12 h). FESEM data demonstrated that agglomerated clusters grew as an elongated grains which migrated to form web-shaped equiaxed structure and dissected to form individual equiaxed microstructure. With femtosecond laser excitation (800 nm, 150 fs), open aperture Z-scan data revealed the presence of two-photon absorption. The nonlinear refractive index (n2) toggled between positive and negative nonlinearity for different microstructures. Web-shaped equiaxed structure kindled both the nonlinear absorption (βeff = 2.0 × 10-12 m/W), nonlinear refraction (n2 = 3.16 × 10-17 m2/W) and a strong optical limiting action (onset limiting threshold of 22.24 μJ/cm2).
Forward-backward equations for nonlinear propagation in axially invariant optical systems
International Nuclear Information System (INIS)
Ferrando, Albert; Zacares, Mario; Fernandez de Cordoba, Pedro; Binosi, Daniele; Montero, Alvaro
2005-01-01
We present a general framework to deal with forward and backward components of the electromagnetic field in axially invariant nonlinear optical systems, which include those having any type of linear or nonlinear transverse inhomogeneities. With a minimum amount of approximations, we obtain a system of two first-order equations for forward and backward components, explicitly showing the nonlinear couplings among them. The modal approach used allows for an effective reduction of the dimensionality of the original problem from 3+1 (three spatial dimensions plus one time dimension) to 1+1 (one spatial dimension plus one frequency dimension). The new equations can be written in a spinor Dirac-like form, out of which conserved quantities can be calculated in an elegant manner. Finally, these equations inherently incorporate spatiotemporal couplings, so that they can be easily particularized to deal with purely temporal or purely spatial effects. Nonlinear forward pulse propagation and nonparaxial evolution of spatial structures are analyzed as examples
Nonlinear optical properties of Nd3+-Li+ co-doped ZnS-PVP thin films
Talwatkar, S. S.; Sunatkari, A. L.; Tamgadge, Y. S.; Muley, G. G.
2018-04-01
The nonlinear optical properties of Nd3+-Li+ co-doped ZnS-PVP nanocomposite were studied using a continuous wave (CW) He-Ne laser (λ = 632.8 nm)by z-scan technique. The nonlinear refractive index (n2), absorption coefficient (β) and third order nonlinear susceptibility (χ(3)) of PVP thin films embedded with Nd3+-Li+ co-doped ZnS NPs was found in the order of 10-7 cm2/W, 10-6 cm/W and 10-7 esu respectively. The nonlinearity found increasing with Nd3+-Li+ co-dopant concentration. Based on the results, it is proposed that this material is a new class of luminescent material suitable in optoelectronics devices application, especially in light-emitting devices, electroluminescent devices, display devices, etc.
Efficient control of ultrafast optical nonlinearity of reduced graphene oxide by infrared reduction
Energy Technology Data Exchange (ETDEWEB)
Bhattachraya, S.; Maiti, R.; Das, A. C.; Saha, S.; Mondal, S.; Ray, S. K.; Bhaktha, S. N. B.; Datta, P. K., E-mail: pkdatta.iitkgp@gmail.com [Department of Physics, Indian Institute of Technology Kharagpur, Kharagpur 721302 (India)
2016-07-07
Simultaneous occurrence of saturable absorption nonlinearity and two-photon absorption nonlinearity in the same medium is well sought for the devices like optical limiter and laser mode-locker. Pristine graphene sheet consisting entirely of sp{sup 2}-hybridized carbon atoms has already been identified having large optical nonlinearity. However, graphene oxide (GO), a precursor of graphene having both sp{sup 2} and sp{sup 3}-hybridized carbon atom, is increasingly attracting cross-discipline researchers for its controllable properties by reduction of oxygen containing groups. In this work, GO has been prepared by modified Hummers method, and it has been further reduced by infrared (IR) radiation. Characterization of reduced graphene oxide (RGO) by means of Raman spectroscopy, X-ray photoelectron spectroscopy, and UV-Visible absorption measurements confirms an efficient reduction with infrared radiation. Here, we report precise control of non-linear optical properties of RGO in femtosecond regime with increased degrees of IR reduction measured by open aperture z-scan technique. Depending on the intensity, both saturable absorption and two-photon absorption effects are found to contribute to the non-linearity of all the samples. Saturation dominates at low intensity (∼127 GW/cm{sup 2}) while two-photon absorption becomes prominent at higher intensities (from 217 GW/cm{sup 2} to 302 GW/cm{sup 2}). The values of two-photon absorption co-efficient (∼0.0022–0.0037 cm/GW for GO, and ∼0.0128–0.0143 cm/GW for RGO) and the saturation intensity (∼57 GW/cm{sup 2} for GO, and ∼194 GW/cm{sup 2} for RGO) increase with increasing reduction, indicating GO and RGO as novel tunable photonic devices. We have also explained the reason of tunable nonlinear optical properties by using amorphous carbon model.
Efficient control of ultrafast optical nonlinearity of reduced graphene oxide by infrared reduction
International Nuclear Information System (INIS)
Bhattachraya, S.; Maiti, R.; Das, A. C.; Saha, S.; Mondal, S.; Ray, S. K.; Bhaktha, S. N. B.; Datta, P. K.
2016-01-01
Simultaneous occurrence of saturable absorption nonlinearity and two-photon absorption nonlinearity in the same medium is well sought for the devices like optical limiter and laser mode-locker. Pristine graphene sheet consisting entirely of sp"2-hybridized carbon atoms has already been identified having large optical nonlinearity. However, graphene oxide (GO), a precursor of graphene having both sp"2 and sp"3-hybridized carbon atom, is increasingly attracting cross-discipline researchers for its controllable properties by reduction of oxygen containing groups. In this work, GO has been prepared by modified Hummers method, and it has been further reduced by infrared (IR) radiation. Characterization of reduced graphene oxide (RGO) by means of Raman spectroscopy, X-ray photoelectron spectroscopy, and UV-Visible absorption measurements confirms an efficient reduction with infrared radiation. Here, we report precise control of non-linear optical properties of RGO in femtosecond regime with increased degrees of IR reduction measured by open aperture z-scan technique. Depending on the intensity, both saturable absorption and two-photon absorption effects are found to contribute to the non-linearity of all the samples. Saturation dominates at low intensity (∼127 GW/cm"2) while two-photon absorption becomes prominent at higher intensities (from 217 GW/cm"2 to 302 GW/cm"2). The values of two-photon absorption co-efficient (∼0.0022–0.0037 cm/GW for GO, and ∼0.0128–0.0143 cm/GW for RGO) and the saturation intensity (∼57 GW/cm"2 for GO, and ∼194 GW/cm"2 for RGO) increase with increasing reduction, indicating GO and RGO as novel tunable photonic devices. We have also explained the reason of tunable nonlinear optical properties by using amorphous carbon model.
All-Optical Control of Linear and Nonlinear Energy Transfer via the Zeno Effect
Guo, Xiang; Zou, Chang-Ling; Jiang, Liang; Tang, Hong X.
2018-05-01
Microresonator-based nonlinear processes are fundamental to applications including microcomb generation, parametric frequency conversion, and harmonics generation. While nonlinear processes involving either second- (χ(2 )) or third- (χ(3 )) order nonlinearity have been extensively studied, the interaction between these two basic nonlinear processes has seldom been reported. In this paper we demonstrate a coherent interplay between second- and third- order nonlinear processes. The parametric (χ(2 ) ) coupling to a lossy ancillary mode shortens the lifetime of the target photonic mode and suppresses its density of states, preventing the photon emissions into the target photonic mode via the Zeno effect. Such an effect is then used to control the stimulated four-wave mixing process and realize a suppression ratio of 34.5.
Directory of Open Access Journals (Sweden)
Tamer Ömer
2016-03-01
Full Text Available The molecular modeling of p-nitroanilinium perchlorate molecule was carried out by using B3LYP and HSEH1PBE levels of density functional theory (DFT. The IR and Raman spectra were simulated and the assignments of vibrational modes were performed on the basis of relative contribution of various internal co-ordinates. NBO analysis was performed to demonstrate charge transfer, conjugative interactions and the formation of intramolecular hydrogen bonding interactions within PNAPC. Obtained large dipole moment values showed that PNAPC is a highly polarizable complex, and the charge transfer occurs within PNAPC. Hydrogen bonding and charge transfer interactions were also displayed by small HOMO-LUMO gap and molecular electrostatic potential (MEP surface. The strong evidences that the material can be used as an efficient nonlinear optical (NLO material of PNAPC were demonstrated by considerable polarizability and hyperpolarizability values obtained at DFT levels.
Rate of non-linearity in DMS aerosol-cloud-climate interactions
Directory of Open Access Journals (Sweden)
M. A. Thomas
2011-11-01
Full Text Available The degree of non-linearity in DMS-cloud-climate interactions is assessed using the ECHAM5-HAMMOZ model by taking into account end-to-end aerosol chemistry-cloud microphysics link. The evaluation is made over the Southern oceans in austral summer, a region of minimal anthropogenic influence. In this study, we compare the DMS-derived changes in the aerosol and cloud microphysical properties between a baseline simulation with the ocean DMS emissions from a prescribed climatology, and a scenario where the DMS emissions are doubled. Our results show that doubling the DMS emissions in the current climate results in a non-linear response in atmospheric DMS burden and subsequently, in SO_{2} and H_{2}SO_{4} burdens due to inadequate OH oxidation. The aerosol optical depth increases by only ~20 % in the 30° S–75° S belt in the SH summer months. This increases the vertically integrated cloud droplet number concentrations (CDNC by 25 %. Since the vertically integrated liquid water vapor is constant in our model simulations, an increase in CDNC leads to a reduction in cloud droplet radius of 3.4 % over the Southern oceans in summer. The equivalent increase in cloud liquid water path is 10.7 %. The above changes in cloud microphysical properties result in a change in global annual mean radiative forcing at the TOA of −1.4 W m^{−2}. The results suggest that the DMS-cloud microphysics link is highly non-linear. This has implications for future studies investigating the DMS-cloud climate feedbacks in a warming world and for studies evaluating geoengineering options to counteract warming by modulating low level marine clouds.
Heteroepitaxy of orientation-patterned nonlinear optical materials
Tassev, Vladimir L.; Vangala, Shivashankar R.; Peterson, Rita D.; Snure, Michael
2018-03-01
We report some recent results on thick heteroepitaxial growth of GaP on GaAs substrates and on orientation-patterned (OP) GaAs templates conducted in a hot-wall horizontal quartz reactor for Hydride Vapor Phase Epitaxy. The growths on the plain substrates resulted in up to 500 μm thick GaP with smooth surface morphology (RMS following stages of growth, as well on the mechanisms of the strain relaxation from the lattice and thermal mismatch between layer and substrate. The efforts to accommodate the growing film to the foreign substrate by engineering an intermediate buffer layer were extended to thick growths of GaAsxP1-x ternary with the idea to combine in one material the best of the nonlinear properties of GaP and GaAs that are strictly relevant to the pursued applications.
Model-free inference of direct network interactions from nonlinear collective dynamics.
Casadiego, Jose; Nitzan, Mor; Hallerberg, Sarah; Timme, Marc
2017-12-19
The topology of interactions in network dynamical systems fundamentally underlies their function. Accelerating technological progress creates massively available data about collective nonlinear dynamics in physical, biological, and technological systems. Detecting direct interaction patterns from those dynamics still constitutes a major open problem. In particular, current nonlinear dynamics approaches mostly require to know a priori a model of the (often high dimensional) system dynamics. Here we develop a model-independent framework for inferring direct interactions solely from recording the nonlinear collective dynamics generated. Introducing an explicit dependency matrix in combination with a block-orthogonal regression algorithm, the approach works reliably across many dynamical regimes, including transient dynamics toward steady states, periodic and non-periodic dynamics, and chaos. Together with its capabilities to reveal network (two point) as well as hypernetwork (e.g., three point) interactions, this framework may thus open up nonlinear dynamics options of inferring direct interaction patterns across systems where no model is known.
Impurity-defect induced noncentrosymmetricity in nonlinear optical processes
International Nuclear Information System (INIS)
Miah, M. Idrish
2009-01-01
Noncentrosymmetric nanosize-material processes in cadmium iodide are formed by doping it with the impurity copper. The noncentrosymmetricity in the processes are probed by the observation of the second-order optical susceptibility χ ijk (2) . The value of χ ijk (2) is found to depend fashionably on the impurity content of the nanomaterials. The results also show that a significant enhancement in the noncentrosymmetric response is achieved in nanomaterials with reduced sizes and at low temperatures.
Linear and nonlinear optical properties of a hydrogenic donor in lens-shaped quantum dots
International Nuclear Information System (INIS)
Vahdani, M.R.K.; Rezaei, G.
2009-01-01
Optical transitions in a Lens-Shaped Quantum Dot (LSD) are investigated in the presence of a hydrogenic impurity. The electronic wave functions are obtained analytically and the energy eigenvalues are calculated numerically. The density matrix formulation with the intersubband relaxation are used to evaluate the (linear and third order nonlinear) absorption coefficient (AC) and the change in the refractive indices (RI) analytically. The effect of the size of the LSD and optical intensity on the AC and RI are investigated. It is found that AC and RI are strongly affected by the optical intensity and the size of the LSD.
Linear and nonlinear optical properties of a hydrogenic donor in lens-shaped quantum dots
Energy Technology Data Exchange (ETDEWEB)
Vahdani, M.R.K. [Department of Physics, College of Sciences, Shiraz University, Shiraz 71454 (Iran, Islamic Republic of); Rezaei, G., E-mail: grezaei@mail.yu.ac.i [Department of Physics, College of Sciences, Yasouj University, Yasouj 75914 (Iran, Islamic Republic of)
2009-08-17
Optical transitions in a Lens-Shaped Quantum Dot (LSD) are investigated in the presence of a hydrogenic impurity. The electronic wave functions are obtained analytically and the energy eigenvalues are calculated numerically. The density matrix formulation with the intersubband relaxation are used to evaluate the (linear and third order nonlinear) absorption coefficient (AC) and the change in the refractive indices (RI) analytically. The effect of the size of the LSD and optical intensity on the AC and RI are investigated. It is found that AC and RI are strongly affected by the optical intensity and the size of the LSD.
Communication: atomic force detection of single-molecule nonlinear optical vibrational spectroscopy.
Saurabh, Prasoon; Mukamel, Shaul
2014-04-28
Atomic Force Microscopy (AFM) allows for a highly sensitive detection of spectroscopic signals. This has been first demonstrated for NMR of a single molecule and recently extended to stimulated Raman in the optical regime. We theoretically investigate the use of optical forces to detect time and frequency domain nonlinear optical signals. We show that, with proper phase matching, the AFM-detected signals closely resemble coherent heterodyne-detected signals. Applications are made to AFM-detected and heterodyne-detected vibrational resonances in Coherent Anti-Stokes Raman Spectroscopy (χ((3))) and sum or difference frequency generation (χ((2))).
Interferometric and nonlinear-optical spectral-imaging techniques for outer space and live cells
Itoh, Kazuyoshi
2015-12-01
Multidimensional signals such as the spectral images allow us to have deeper insights into the natures of objects. In this paper the spectral imaging techniques that are based on optical interferometry and nonlinear optics are presented. The interferometric imaging technique is based on the unified theory of Van Cittert-Zernike and Wiener-Khintchine theorems and allows us to retrieve a spectral image of an object in the far zone from the 3D spatial coherence function. The retrieval principle is explained using a very simple object. The promising applications to space interferometers for astronomy that are currently in progress will also be briefly touched on. An interesting extension of interferometric spectral imaging is a 3D and spectral imaging technique that records 4D information of objects where the 3D and spectral information is retrieved from the cross-spectral density function of optical field. The 3D imaging is realized via the numerical inverse propagation of the cross-spectral density. A few techniques suggested recently are introduced. The nonlinear optical technique that utilizes stimulated Raman scattering (SRS) for spectral imaging of biomedical targets is presented lastly. The strong signals of SRS permit us to get vibrational information of molecules in the live cell or tissue in real time. The vibrational information of unstained or unlabeled molecules is crucial especially for medical applications. The 3D information due to the optical nonlinearity is also the attractive feature of SRS spectral microscopy.
Synthesis of polymeric micro- and nanostructural materials for application in non-linear optics
International Nuclear Information System (INIS)
Kravets, Lyubov; Palistrant, Natalia; Bivol, Valerii; Robu, Stepan; Barba, Nikolai; Orelovitch, Oleg
2007-01-01
The present paper describes a new approach developed for the preparation of micro- and nanostructural materials on the basis of polymeric compositions used as a matrix in non-linear optics. This approach consists in filling the pores of poly(ethylene terephthalate) track membranes (PET TM) from polymeric compositions using an impregnation method. It is shown that depending on the concentration of polymeric compositions in the solution it is possible to form a variety of micro- and nanostructural materials (tubules and wires as well as composite membranes) with a wide spectrum of characteristics. The developed method of producing micro- and nanostructural materials provides a possible way for creating polymeric objects with non-linear optic properties which can be used to design electronic micro- and nanodevices and to obtain chemical and optical sensors