Focusing coherent light through a nonlinear scattering medium
Frostig, Hadas; Derevyanko, Stanislav; Silberberg, Yaron
2016-01-01
Wavefront shaping is a powerful technique that can be used to focus light through scattering media, with the limitation that the obtained focus contains a small fraction of the total power. The method is based on the assumption that the field at the output is a linear superposition of the modes traveling through different paths in the medium. However, when the scattering medium also exhibits nonlinearity, as may occur in multiphoton microscopy, this assumption is violated and the applicability of wavefront shaping becomes unclear. Here we show that using adaptive optimization of the wavefront light can still be controlled and focused through a nonlinear scattering medium, and that the focused fraction of power can be significantly enhanced in the presence of moderate positive nonlinearity. Our results suggest that the use of short pulses for focusing through scattering media with a mild self-focusing response might be favorable to the use of continuous-wave light.
Gamma ray vortices from nonlinear inverse Compton scattering of circularly polarized light
Taira, Yoshitaka; Katoh, Masahiro
2016-01-01
Inverse Compton scattering (ICS) is an elemental radiation process that produces high-energy photons both in nature and in the laboratory. Non-linear ICS is a process in which multiple photons are converted to a single high-energy photon. Here, we theoretically show that the photon produced by non-linear ICS of circularly polarized photons is a vortex, which means that it possesses a helical wave front and carries orbital angular momentum. Our work explains a recent experimental result regarding non-linear Compton scattering that clearly shows an annular intensity distribution as a remarkable feature of a vortex beam. Our work implies that gamma ray vortices should be produced in various situations in astrophysics in which high-energy electrons and intense circularly polarized light fields coexist. They should play a critical role in stellar nucleosynthesis. Non-linear ICS is the most promising radiation process for realizing a gamma ray vortex source based on currently available laser and accelerator technol...
Particle sizing by dynamic light scattering: non-linear cumulant analysis.
Mailer, Alastair G; Clegg, Paul S; Pusey, Peter N
2015-04-15
We revisit the method of cumulants for analysing dynamic light scattering data in particle sizing applications. Here the data, in the form of the time correlation function of scattered light, is written as a series involving the first few cumulants (or moments) of the distribution of particle diffusion constants. Frisken (2001 Appl. Opt. 40 4087) has pointed out that, despite greater computational complexity, a non-linear, iterative, analysis of the data has advantages over the linear least-squares analysis used originally. In order to explore further the potential and limitations of cumulant methods we analyse, by both linear and non-linear methods, computer-generated data with realistic 'noise', where the parameters of the distribution can be set explicitly. We find that, with modern computers, non-linear analysis is straightforward and robust. The mean and variance of the distribution of diffusion constants can be obtained quite accurately for distributions of width (standard deviation/mean) up to about 0.6, but there appears to be little prospect of obtaining meaningful higher moments.
Nonlinear scattering in plasmonic nanostructures
Chu, Shi-Wei
2016-09-01
Nonlinear phenomena provide novel light manipulation capabilities and innovative applications. Recently, we discovered nonlinear saturation on single-particle scattering of gold nanospheres by continuous-wave laser excitation and innovatively applied to improve microscopic resolution down to λ/8. However, the nonlinearity was limited to the green-orange plasmonic band of gold nanosphere, and the underlying mechanism has not yet been fully understood. In this work, we demonstrated that nonlinear scattering exists for various material/geometry combinations, thus expanding the applicable wavelength range. For near-infrared, gold nanorod is used, while for blue-violet, silver nanospheres are adopted. In terms of mechanism, the nonlinearity may originate from interband/intraband absorption, hot electron, or hot lattice, which are spectrally mixed in the case of gold nanosphere. For gold nanorod and silver nanosphere, nonlinear scattering occurs at plasmonic resonances, which are spectrally far from interband/intraband absorptions, so they are excluded. We found that the nonlinear index is much larger than possible contributions from hot electrons in literature. Therefore, we conclude that hot lattice is the major mechanism. In addition, we propose that similar to z-scan, which is the standard method to characterize nonlinearity of a thin sample, laser scanning microscopy should be adopted as the standard method to characterize nonlinearity from a nanostructure. Our work not only provides the physical mechanism of the nonlinear scattering, but also paves the way toward multi-color superresolution imaging based on non-bleaching plasmonic scattering.
Observation of Nonlinear Compton Scattering
Energy Technology Data Exchange (ETDEWEB)
Kotseroglou, T.
2003-12-19
This experiment tests Quantum Electrodynamics in the strong field regime. Nonlinear Compton scattering has been observed during the interaction of a 46.6 GeV electron beam with a 10{sup 18} W/cm{sup 2} laser beam. The strength of the field achieved was measured by the parameter {eta} = e{var_epsilon}{sub rms}/{omega}mc = 0.6. Data were collected with infrared and green laser photons and circularly polarized laser light. The timing stabilization achieved between the picosecond laser and electron pulses has {sigma}{sub rms} = 2 ps. A strong signal of electrons that absorbed up to 4 infrared photons (or up to 3 green photons) at the same point in space and time, while emitting a single gamma ray, was observed. The energy spectra of the scattered electrons and the nonlinear dependence of the electron yield on the field strength agreed with the simulation over 3 orders of magnitude. The detector could not resolve the nonlinear Compton scattering from the multiple single Compton scattering which produced rates of scattered electrons of the same order of magnitude. Nevertheless, a simulation has studied this difference and concluded that the scattered electron rates observed could not be accounted for only by multiple ordinary Compton scattering; nonlinear Compton scattering processes are dominant for n {ge} 3.
Galaĭchuk, Yu A.; Yashkir, Yu N.
1989-12-01
A theory is developed for the calculation of the gain g due to stimulated resonant hyper-Raman scattering of light by polaritons in gaseous media. It is shown that throughout the tuning range of the pump frequency (including one- and two-photon resonances) a maximum of g corresponds to a dispersion curve of polaritons plotted ignoring attenuation. Theoretical results are used to analyze characteristics of hyper-Raman scattering in sodium vapor. It is shown that under normal experimental conditions the splitting of polariton branches is considerable (amounting to tens of reciprocal centimeters on the frequency scale and several angular degrees). The value of g is estimated for two-photon resonances in the case when the pump frequency is tunable in a wide range. The optimal conditions for stimulated hyper-Raman scattering are identified.
J. Puķīte; T. Wagner
2016-01-01
We address the application of differential optical absorption spectroscopy (DOAS) of scattered light observations in the presence of strong absorbers (in particular ozone), for which the absorption optical depth is a non-linear function of the trace gas concentration. This is the case because Beer–Lambert law generally does not hold for scattered light measurements due to many light paths contributing to the measurement. While in many cases linear approximation can be made, ...
Incoherent subharmonic light scattering in isotropic media.
Feng, D H; Xu, Z Z; Feng, X L; Jia, T Q; Li, X X; Liu, J S
2005-02-01
Incoherent subharmonic light scattering in isotropic media is a new kind of nonlinear light scattering, which involves single input photon and multiple output photons of equal frequency. We investigate theoretically the dependence of the subharmonic scattering intensity on the hyperpolarizability of molecules and the incident intensity using nonlinear optics theory similar to that used for Hyper-Rayleigh scattering and degenerate optical parametric oscillators. It is derived that the subharmonic scattering intensities grow exponentially or superexponentially with the hyperpolarizability of molecules and the incident intensity.
Puķīte, Jānis; Wagner, Thomas
2016-05-01
We address the application of differential optical absorption spectroscopy (DOAS) of scattered light observations in the presence of strong absorbers (in particular ozone), for which the absorption optical depth is a non-linear function of the trace gas concentration. This is the case because Beer-Lambert law generally does not hold for scattered light measurements due to many light paths contributing to the measurement. While in many cases linear approximation can be made, for scenarios with strong absorptions non-linear effects cannot always be neglected. This is especially the case for observation geometries, for which the light contributing to the measurement is crossing the atmosphere under spatially well-separated paths differing strongly in length and location, like in limb geometry. In these cases, often full retrieval algorithms are applied to address the non-linearities, requiring iterative forward modelling of absorption spectra involving time-consuming wavelength-by-wavelength radiative transfer modelling. In this study, we propose to describe the non-linear effects by additional sensitivity parameters that can be used e.g. to build up a lookup table. Together with widely used box air mass factors (effective light paths) describing the linear response to the increase in the trace gas amount, the higher-order sensitivity parameters eliminate the need for repeating the radiative transfer modelling when modifying the absorption scenario even in the presence of a strong absorption background. While the higher-order absorption structures can be described as separate fit parameters in the spectral analysis (so-called DOAS fit), in practice their quantitative evaluation requires good measurement quality (typically better than that available from current measurements). Therefore, we introduce an iterative retrieval algorithm correcting for the higher-order absorption structures not yet considered in the DOAS fit as well as the absorption dependence on
Inelastic Light Scattering Processes
Fouche, Daniel G.; Chang, Richard K.
1973-01-01
Five different inelastic light scattering processes will be denoted by, ordinary Raman scattering (ORS), resonance Raman scattering (RRS), off-resonance fluorescence (ORF), resonance fluorescence (RF), and broad fluorescence (BF). A distinction between fluorescence (including ORF and RF) and Raman scattering (including ORS and RRS) will be made in terms of the number of intermediate molecular states which contribute significantly to the scattered amplitude, and not in terms of excited state lifetimes or virtual versus real processes. The theory of these processes will be reviewed, including the effects of pressure, laser wavelength, and laser spectral distribution on the scattered intensity. The application of these processes to the remote sensing of atmospheric pollutants will be discussed briefly. It will be pointed out that the poor sensitivity of the ORS technique cannot be increased by going toward resonance without also compromising the advantages it has over the RF technique. Experimental results on inelastic light scattering from I(sub 2) vapor will be presented. As a single longitudinal mode 5145 A argon-ion laser line was tuned away from an I(sub 2) absorption line, the scattering was observed to change from RF to ORF. The basis, of the distinction is the different pressure dependence of the scattered intensity. Nearly three orders of magnitude enhancement of the scattered intensity was measured in going from ORF to RF. Forty-seven overtones were observed and their relative intensities measured. The ORF cross section of I(sub 2) compared to the ORS cross section of N2 was found to be 3 x 10(exp 6), with I(sub 2) at its room temperature vapor pressure.
Arditi, Tal; Granot, Er'el; Sternklar, Shmuel
2007-09-15
Brillouin amplification with counterpropagating modulated pump and Stokes light leads to nonlinear modulation-phase shifts of the interacting intensity waves. This is due to a partial transformation of the nonmodulated light component at the input into modulated light at the output as a result of a mixing process with the counterpropagating modulated component of the pump and results in an advance or delay of the input modulation. This occurs for interactions over less than half of a modulation wavelength. Milliwatts of power in a kilometer of standard single-mode fiber give significant tunability of the modulation phase.
Energy Technology Data Exchange (ETDEWEB)
Quaglioni, S; Navratil, P; Roth, R
2009-12-15
The exact treatment of nuclei starting from the constituent nucleons and the fundamental interactions among them has been a long-standing goal in nuclear physics. Above all nuclear scattering and reactions, which require the solution of the many-body quantum-mechanical problem in the continuum, represent an extraordinary theoretical as well as computational challenge for ab initio approaches.We present a new ab initio many-body approach which derives from the combination of the ab initio no-core shell model with the resonating-group method [4]. By complementing a microscopic cluster technique with the use of realistic interactions, and a microscopic and consistent description of the nucleon clusters, this approach is capable of describing simultaneously both bound and scattering states in light nuclei. We will discuss applications to neutron and proton scattering on sand light p-shell nuclei using realistic nucleon-nucleon potentials, and outline the progress toward the treatment of more complex reactions.
Light scattering reviews 8 radiative transfer and light scattering
Kokhanovsky, Alexander A
2013-01-01
Light scattering review (vol 8) is aimed at the presentation of recent advances in radiative transfer and light scattering optics. The topics to be covered include: scattering of light by irregularly shaped particles suspended in atmosphere (dust, ice crystals), light scattering by particles much larger as compared the wavelength of incident radiation, atmospheric radiative forcing, astrophysical radiative transfer, radiative transfer and optical imaging in biological media, radiative transfer of polarized light, numerical aspects of radiative transfer.
Wahle, Chris W; Ross, David S; Thurston, George M
2012-07-21
We mathematically design sets of static light scattering experiments to provide for model-independent measurements of ternary liquid mixing free energies to a desired level of accuracy. A parabolic partial differential equation (PDE), linearized from the full nonlinear PDE [D. Ross, G. Thurston, and C. Lutzer, J. Chem. Phys. 129, 064106 (2008)], describes how data noise affects the free energies to be inferred. The linearized PDE creates a net of spacelike characteristic curves and orthogonal, timelike curves in the composition triangle, and this net governs diffusion of information coming from light scattering measurements to the free energy. Free energy perturbations induced by a light scattering perturbation diffuse along the characteristic curves and towards their concave sides, with a diffusivity that is proportional to the local characteristic curvature radius. Consequently, static light scattering can determine mixing free energies in regions with convex characteristic curve boundaries, given suitable boundary data. The dielectric coefficient is a Lyapunov function for the dynamical system whose trajectories are PDE characteristics. Information diffusion is heterogeneous and system-dependent in the composition triangle, since the characteristics depend on molecular interactions and are tangent to liquid-liquid phase separation coexistence loci at critical points. We find scaling relations that link free energy accuracy, total measurement time, the number of samples, and the interpolation method, and identify the key quantitative tradeoffs between devoting time to measuring more samples, or fewer samples more accurately. For each total measurement time there are optimal sample numbers beyond which more will not improve free energy accuracy. We estimate the degree to which many-point interpolation and optimized measurement concentrations can improve accuracy and save time. For a modest light scattering setup, a sample calculation shows that less than two
Nonlinear X-ray Compton Scattering
Fuchs, Matthias; Chen, Jian; Ghimire, Shambhu; Shwartz, Sharon; Kozina, Michael; Jiang, Mason; Henighan, Thomas; Bray, Crystal; Ndabashimiye, Georges; Bucksbaum, P H; Feng, Yiping; Herrmann, Sven; Carini, Gabriella; Pines, Jack; Hart, Philip; Kenney, Christopher; Guillet, Serge; Boutet, Sebastien; Williams, Garth; Messerschmidt, Marc; Seibert, Marvin; Moeller, Stefan; Hastings, Jerome B; Reis, David A
2015-01-01
X-ray scattering is a weak linear probe of matter. It is primarily sensitive to the position of electrons and their momentum distribution. Elastic X-ray scattering forms the basis of atomic structural determination while inelastic Compton scattering is often used as a spectroscopic probe of both single-particle excitations and collective modes. X-ray free-electron lasers (XFELs) are unique tools for studying matter on its natural time and length scales due to their bright and coherent ultrashort pulses. However, in the focus of an XFEL the assumption of a weak linear probe breaks down, and nonlinear light-matter interactions can become ubiquitous. The field can be sufficiently high that even non-resonant multiphoton interactions at hard X-rays wavelengths become relevant. Here we report the observation of one of the most fundamental nonlinear X-ray-matter interactions, the simultaneous Compton scattering of two identical photons producing a single photon at nearly twice the photon energy. We measure scattered...
Light scattering by small particles
Hulst, H C van de
1981-01-01
""A must for researchers using the techniques of light scattering."" ? S. C. Snowdon, Journal of the Franklin InstituteThe measurement of light scattering of independent, homogeneous particles has many useful applications in physical chemistry, meteorology and astronomy. There is, however, a sizeable gap between the abstract formulae related to electromagnetic-wave-scattering phenomena, and the computation of reliable figures and curves. Dr. van de Hulst's book enables researchers to bridge that gap. The product of twelve years of work, it is an exhaustive study of light-scattering properties
Light scattering reviews 9 light scattering and radiative transfer
Kokhanovsky, Alexander A
2014-01-01
This book details modern methods of the radiative transfer theory. It presents recent advances in light scattering (measurements and theory) and highlights the newest developments in remote sensing of aerosol and cloud properties.
Scattering of light by crystals
Hayes, William
2012-01-01
This authoritative graduate-level text describes inelastic light scattering by crystals and its use in the investigation of solid-state excitation, with experimental techniques common to all types of excitation. 1978 edition.
Cardona, Manuel
2007-01-01
This is the ninth volume of a well-established series in which expert practitioners discuss topical aspects of light scattering in solids. It reviews recent developments concerning mainly semiconductor nanostructures and inelastic x-ray scattering, including both coherent time-domain and spontaneous scattering studies. In the past few years, light scattering has become one of the most important research and characterization methods for studying carbon nanotubes and semiconducting quantum dots, and a crucial tool for exploring the coupled exciton--photon system in semiconductor cavities. Among the novel techniques discussed in this volume are pump--probe ultrafast measurements and those which use synchrotron radiation as light source. The book addresses improvements in the intensity, beam quality and time synchronization of modern synchrotron sources, which made it possible to measure the phonon dispersion in very small samples and to determine electronic energy bands as well as enabling real-time observations...
Light repolarization by scattering media
Sorrentini, Jacques; Soriano, Gabriel; Amra, Claude
2011-01-01
The polarization of a coherent depolarized incident light beam passing through a disordered medium is investigated. The local polarization of the scattered far field and the probability density function are calculated and show an excellent agreement with experiment. It is demonstrated that complex media may confer high degree of polarization (0.75 DOP average) to the incident unpolarized light.
Laser light scattering basic principles and practice
Chu, Benjamin
1994-01-01
Geared toward upper-level undergraduate and graduate students, this text introduces the interdisciplinary area of laser light scattering, focusing chiefly on theoretical concepts of quasielastic laser scattering.
Nonlinear Light-Matter Interactions in Metamaterials
O'Brien, Kevin Patrick
Metamaterials possess extraordinary linear optical properties never observed in natural materials such as a negative refractive index, enabling exciting applications such as super resolution imaging and cloaking. In this thesis, we explore the equally extraordinary nonlinear properties of metamaterials. Nonlinear optics, the study of light-matter interactions where the optical fields are strong enough to change material properties, has fundamental importance to physics, chemistry, and material science as a non-destructive probe of material properties and has important technological applications such as entangled photon generation and frequency conversion. Due to their ability to manipulate both linear and nonlinear light matter interactions through sub-wavelength structuring, metamaterials are a promising direction for both fundamental and applied nonlinear optics research. We perform the first experiments on nonlinear propagation in bulk zero and negative index optical metamaterials and demonstrate that a zero index material can phase match four wave mixing processes in ways not possible in finite index materials. In addition, we demonstrate the ability of nonlinear scattering theory to describe the geometry dependence of second and third harmonic generation in plasmonic nanostructures. As an application of nonlinear metamaterials, we propose a phase matching technique called "resonant phase matching" to increase the gain and bandwidth of Josephson junction traveling wave parametric amplifiers. With collaborators, we demonstrate a best in class amplifier for superconducting qubit readout--over 20 dB gain with near quantum limited noise performance with a bandwidth and dynamic range an order of magnitude larger than alternative devices. In conclusion, we have demonstrated several ways in which nonlinear metamaterials surpass their natural counterparts. We look forward to the future of the field where nonlinear and quantum metamaterials will enable further new
Light Scattering in Exoplanet Transits
Robinson, Tyler D.; Fortney, Jonathan J.
2016-10-01
Transit spectroscopy is currently the leading technique for studying exoplanet atmospheric composition, and has led to the detection of molecular species, clouds, and/or hazes for numerous worlds outside the Solar System. The field of exoplanet transit spectroscopy will be revolutionized with the anticipated launch of NASA's James Webb Space Telescope (JWST) in 2018. Over the course of the design five year mission for JWST, the observatory is expected to provide in-depth observations of many tens of transiting exoplanets, including some worlds in the poorly understood 2-4 Earth-mass regime. As the quality of transit spectrum observations continues to improve, so should models of exoplanet transits. Thus, certain processes initially thought to be of second-order importance should be revisited and possibly added to modeling tools. For example, atmospheric refraction, which was commonly omitted from early transit spectrum models, has recently been shown to be of critical importance in some terrestrial exoplanet transits. Beyond refraction, another process that has seen little study with regards to exoplanet transits is light multiple scattering. In most cases, scattering opacity in exoplanet transits has been treated as equivalent to absorption opacity. However, this equivalence cannot always hold, such as in the case of a strongly forward scattering, weakly absorbing aerosol. In this presentation, we outline a theory of exoplanet transit spectroscopy that spans the geometric limit (used in most modern models) to a fully multiple scattering approach. We discuss a new technique for improving model efficiency that effectively separates photon paths, which tend to vary slowly in wavelength, from photon absorption, which can vary rapidly in wavelength. Using this newly developed approach, we explore situations where cloud or haze scattering may be important to JWST observations of gas giants, and comment on the conditions necessary for scattering to become a major
Higher-dimensional catastrophes in nonlinear Compton scattering
Kharin, Vasily; Seipt, Daniel; Rykovanov, Sergey
2016-10-01
The Compton scattering of the light on the accelerated electron beam is a valuable tool for generating tunable wide range X- and γ-radiation.However, the cross-section of the scattering is relatively low. That is, in order to obtain bright X-rays one naturally may consider increasing the intensity of the incident light. Passing to relativistic values of laser intensity significantly changes scattering mechanism. Precise QED analysis of the scattered spectra leads to the study of the corresponding elements of S-matrix. Evaluation is usually performed numerically (except cases of specific pulse shapes and scattering angles). We argue that the problem of extracting the scattered spectra in nonlinear Compton scattering of the pulse can be reformulated in terms of studying properties of projection map of specific surfaces associated to the pulse. They are stable with respect to initial conditions, and the brightest regions of the spectrum appear to be in correspondence with the singularities of the projection map, also known as caustics in pure mathematics, diffraction optics and cosmology. Work was supported by the Helmholtz Association (Helmholtz Young Investigators group VH-NG-1037).
Bubble nonlinear dynamics and stimulated scattering process
Jie, Shi; De-Sen, Yang; Sheng-Guo, Shi; Bo, Hu; Hao-Yang, Zhang; Shi-Yong, Hu
2016-02-01
A complete understanding of the bubble dynamics is deemed necessary in order to achieve their full potential applications in industry and medicine. For this purpose it is first needed to expand our knowledge of a single bubble behavior under different possible conditions including the frequency and pressure variations of the sound field. In addition, stimulated scattering of sound on a bubble is a special effect in sound field, and its characteristics are associated with bubble oscillation mode. A bubble in liquid can be considered as a representative example of nonlinear dynamical system theory with its resonance, and its dynamics characteristics can be described by the Keller-Miksis equation. The nonlinear dynamics of an acoustically excited gas bubble in water is investigated by using theoretical and numerical analysis methods. Our results show its strongly nonlinear behavior with respect to the pressure amplitude and excitation frequency as the control parameters, and give an intuitive insight into stimulated sound scattering on a bubble. It is seen that the stimulated sound scattering is different from common dynamical behaviors, such as bifurcation and chaos, which is the result of the nonlinear resonance of a bubble under the excitation of a high amplitude acoustic sound wave essentially. The numerical analysis results show that the threshold of stimulated sound scattering is smaller than those of bifurcation and chaos in the common condition. Project supported by the Program for Changjiang Scholars and Innovative Research Team in University, China (Grant No. IRT1228) and the Young Scientists Fund of the National Natural Science Foundation of China (Grant Nos. 11204050 and 11204049).
UV Nano-Lights - Nonlinear Quantum Dot-Plasmon Coupling
2016-06-20
nanomaterials systems for nonlinear optics. PROJECT TIMELINE The project timeline was segmented into 3 monthly intervals. The PhD students, assisted by...technique to remove the scattering component of light from the fluorescence emission with commonly-used fluorometers [Shortell, Optics Express...nanostructure light interaction and also has helped understand and remove unwanted signal contamination through optical element interference effects as
Light scattering near phase transitions
Cummins, HZ
1983-01-01
Since the development of the laser in the early 1960's, light scattering has played an increasingly crucial role in the investigation of many types of phase transitions and the published work in this field is now widely dispersed in a large number of books and journals.A comprehensive overview of contemporary theoretical and experimental research in this field is presented here. The reviews are written by authors who have actively contributed to the developments that have taken place in both Eastern and Western countries.
Light scattering studies of an electrorheological fluid in oscillatory shear
Energy Technology Data Exchange (ETDEWEB)
Martin, J.E.; Odinek, J.
1995-12-31
We have conducted a real time, two-dimensional light scattering study of the nonlinear dynamics of field-induced structures in an electrorheological fluid subjected to oscillatory shear. We have developed a kinetic chain model of the observed dynamics by considering the response of a fragmenting/aggregating particle chain to the prevailing hydrodynamic and electrostatic forces. This structural theory is then used to describe the nonlinear rheology of ER fluids.
Scattering theory of stochastic electromagnetic light waves.
Wang, Tao; Zhao, Daomu
2010-07-15
We generalize scattering theory to stochastic electromagnetic light waves. It is shown that when a stochastic electromagnetic light wave is scattered from a medium, the properties of the scattered field can be characterized by a 3 x 3 cross-spectral density matrix. An example of scattering of a spatially coherent electromagnetic light wave from a deterministic medium is discussed. Some interesting phenomena emerge, including the changes of the spectral degree of coherence and of the spectral degree of polarization of the scattered field.
Dissipation-induced optical nonlinearity at low light levels
Greenberg, Joel A
2011-01-01
We observe a dissipation-induced nonlinear optical process in a gas of cold atoms that gives rise to large nonlinear coupling strengths with high transparency. The nonlinearity results from the simultaneous cooling and crystallization of the gas, and can give rise to efficient Bragg scattering in the form of a six-wave-mixing process at low-light-levels with an extremely large effective fifth-order nonlinear susceptibility of \\chi^(5)= 7.6 x 10-15 (m/V)^4. For large optical gains, collective scattering due to the strong light-matter coupling leads to slow group velocities (~c/105) and long atomic coherence times (~100 {\\mu}s).
The Amsterdam-Granada Light Scattering Database
Muñoz, O.; Moreno, F.; Guirado, D.; Dabrowska, D.D.; Volten, H.; Hovenier, J.W.
2012-01-01
The Amsterdam Light Scattering Database proved to be a very successful way of promoting the use of the data obtained with the Amsterdam Light Scattering apparatus at optical wavelengths. Many different research groups around the world made use of the experimental data. After the closing down of the
Light scattering on chlorella vulgaris cells
Krol, Tadeusz; Zielinski, Andrzej; Witkowski, Konrad
1992-12-01
Laboratory measurements of light scattering on the axenic cultures of unicellular alga Chlorella vulgaris monoculture confirm the thesis of multi-level light scattering by the cell i.e., both by outer cell membrane and the internal structure of the cell, as well as by its molecular structures. In the measurements, the technique of dynamic light scattering and analysis by the regulation method was used, indicate that the light scattering phenomenon is affected by particles of sizes corresponding either to overall dimensions of the cell or to the dimensions of its internal structures. A correlation was found between the suggested sizes and the stage of physiological evolution of the culture. The measurements of 10 functions constituting the elements of the scattering matrix for an alive Chlorella vulgaris culture and cultures with internal cell structures modified by chemical and mechanical agents evidence that the internal structures of cells play an important role in the interaction of phytoplankton and light.
Properties of nonreciprocal light propagation in a nonlinear optical isolator
Roy, Dibyendu
2016-01-01
Light propagation in a nonlinear optical medium is nonreciprocal for spatially asymmetric linear permittivity. We here examine physical mechanism and properties of such nonreciprocity (NR). For this, we calculate transmission of light through a two-level atom asymmetrically coupled to light inside open waveguides. We determine the critical intensity of incident light for maximum NR and a dependence of the corresponding NR on asymmetry in the coupling. Surprisingly, we find that it is mainly coherent elastic scattering compared to incoherent scattering of incident light which causes maximum NR near the critical intensity. We also show a higher NR of an incident light in the presence of an additional weak light at the opposite port.
Radiofrequency encoded angular-resolved light scattering
DEFF Research Database (Denmark)
Buckley, Brandon W.; Akbari, Najva; Diebold, Eric D.
2015-01-01
The sensitive, specific, and label-free classification of microscopic cells and organisms is one of the outstanding problems in biology. Today, instruments such as the flow cytometer use a combination of light scatter measurements at two distinct angles to infer the size and internal complexity...... of cells at rates of more than 10,000 per second. However, by examining the entire angular light scattering spectrum it is possible to classify cells with higher resolution and specificity. Current approaches to performing these angular spectrum measurements all have significant throughput limitations...... Encoded Angular-resolved Light Scattering (REALS), this technique multiplexes angular light scattering in the radiofrequency domain, such that a single photodetector captures the entire scattering spectrum from a particle over approximately 100 discrete incident angles on a single shot basis. As a proof...
Nonlinear ion acoustic waves scattered by vortexes
Ohno, Yuji; Yoshida, Zensho
2016-09-01
The Kadomtsev-Petviashvili (KP) hierarchy is the archetype of infinite-dimensional integrable systems, which describes nonlinear ion acoustic waves in two-dimensional space. This remarkably ordered system resides on a singular submanifold (leaf) embedded in a larger phase space of more general ion acoustic waves (low-frequency electrostatic perturbations). The KP hierarchy is characterized not only by small amplitudes but also by irrotational (zero-vorticity) velocity fields. In fact, the KP equation is derived by eliminating vorticity at every order of the reductive perturbation. Here, we modify the scaling of the velocity field so as to introduce a vortex term. The newly derived system of equations consists of a generalized three-dimensional KP equation and a two-dimensional vortex equation. The former describes 'scattering' of vortex-free waves by ambient vortexes that are determined by the latter. We say that the vortexes are 'ambient' because they do not receive reciprocal reactions from the waves (i.e., the vortex equation is independent of the wave fields). This model describes a minimal departure from the integrable KP system. By the Painlevé test, we delineate how the vorticity term violates integrability, bringing about an essential three-dimensionality to the solutions. By numerical simulation, we show how the solitons are scattered by vortexes and become chaotic.
Resonance Light Scattering Imaging Determination of Heparin
Institute of Scientific and Technical Information of China (English)
Hong Ping GUO; Cheng Zhi HUANG; Jian LING
2006-01-01
A laser-induced resonance light scattering (RLS) imaging method to determine heparin is described based on the high light scattering emission power of the aggregation species of heparin with α, β, γ, δtetra(4-trimethylaminoniumphenyl)prophyrin (TAPP) in solution. By imaging the light scattering signals of the aggregation species, we proposed the method to determine the heparin with a detection range of 0.02 - 0.6 μg/mL and the detection limit (3 σ) of 1.3 ng/mL.
Transparent alumina: A light scattering model
Apetz, R.; Van Bruggen, P.B.
2003-01-01
A model based on Rayleigh-Gans-Debye light scattering theory has been developed to describe the light transmission properties of fine-grained, fully dense polycrystalline ceramics consisting of birefringent crystals. This model extends light transmission models based on geometrical optics, which are
Investigating Static and Dynamic Light Scattering
Sun, Yong
2011-01-01
A new size, static radii $R_{s}$, can be measured accurately using Static Light Scattering (SLS) technique when the Rayleigh-Gans-Debye approximation is valid for dilute homogenous spherical particles in dispersion. The method proposed in this work not only can measures the particle size distribution and average molar mass accurately but also enables us to explore Dynamic Light Scattering (DLS) technique further. Detailed investigation of the normalized time auto-correlation function of the scattered light intensity $g^{2)}(\\tau)$ shows that the measurements of DLS can be expected accurately and the static and hydrodynamic radii of nanoparticles are different. Only at some special conditions, the Z-average hydrodynamic radius can be measured accurately at a given scattering angle. The fact that the values of average hydrodynamic radius measured at different scattering angles are consistent or the values of polydispersity index are small does not mean the particle size distribution is narrow or monodisperse.
Multiple light scattering in porous gallium phosphide
Bret, Boris Paul Jean
2005-01-01
This thesis presents an experimental study on multiple light scattering, with the necessary introductions: theoretical background and sample preparation. The emphasis is put on the effects of the multiple scattering of waves, i.e., where interference effects exist and are significant, in the search for Anderson localization. In ensemble-averaged random media, there exists a cone of light, superimposed on the diffuse background, in the exact backscattering direction, due to the constructive in...
Scaling up Echo-State Networks with multiple light scattering
Dong, Jonathan; Krzakala, Florent; Wainrib, Gilles
2016-01-01
Echo-State Networks and Reservoir Computing have been studied for more than a decade. As they provide an elegant yet powerful alternative to traditional computing, researchers have tried to implement them using physical systems, in particular non-linear optical elements, achieving high bandwidth and low power consumption. Here we present a completely different optical implementation of Echo-State Networks using light-scattering materials. As a proof of concept, binary networks have been successfully trained to perform non-linear operations on time series and memory of such networks has been evaluated. This new method is fast, power efficient and easily scalable to very large networks.
Nonlinear ion acoustic waves scattered by vortexes
Ohno, Yuji
2015-01-01
The Kadomtsev--Petviashvili (KP) hierarchy is the archetype of infinite-dimensional integrable systems, which describes nonlinear ion acoustic waves in two-dimensional space. This remarkably ordered system resides on a singular submanifold (leaf) embedded in a larger phase space of more general ion acoustic waves (low-frequency electrostatic perturbations). The KP hierarchy is characterized not only by small amplitudes but also by irrotational (zero-vorticity) velocity fields. In fact, the KP equation is derived by eliminating vorticity at every order of the reductive perturbation. Here we modify the scaling of the velocity field so as to introduce a vortex term. The newly derived system of equations consists of a generalized three-dimensional KP equation and a two-dimensional vortex equation. The former describes `scattering' of vortex-free waves by ambient vortexes that are determined by the latter. We say that the vortexes are `ambient' because they do not receive reciprocal reactions from the waves (i.e.,...
Light scattering of interacting gold nanorods
Energy Technology Data Exchange (ETDEWEB)
McGuirt, Baxter; Kielbasa, Jerry; Park, Jung-Ho; Zhang, Junping; Peterson, Eric; Williams, Richard; Carroll, David [Center for Nanotechnology and Molecular Materials and Department of Physics, Wake Forest University, Winston-Salem, NC (United States); Sisco, Patrick; Murphy, Catherine; Adams, Richard D. [Department of Chemistry and Biochemistry, University of South Carolina, Columbia, SC (United States)
2009-12-15
The optical field intensity of light scattering from nanorods of gold has been imaged at distances that are intermediate between the near-field and far-field regimes using a near-field scanning optical microscope (NSOM). For scattering from isolated nanorods the Fraunhofer diffractive behaviour is modified slightly by the dipolar nature of metal nanoantannae as would be expected at these imaging distances. However, when the nanorods are brought into close proximity, interactions between the nanorods alter the scattering behaviour substantially creating large field intensities between the structures. By sampling the field with the near-field microscope tip scanned at different heights, detailed maps of the scattering profile can be generated. The NSOM image of far-field scattered light from an isolated gold nanorod. The nanorod was imaged at a distance of roughly 8 {mu}m above the support substrate using a scanning near-field microscope operated at constant height mode. (Abstract Copyright [2009], Wiley Periodicals, Inc.)
The Whiteness of Things and Light Scattering
Gratton, L. M.; Lopez-Arias, T.; Calza, G.; Oss, S.
2009-01-01
We discuss some simple experiments dealing with intriguing properties of light and its interaction with matter. In particular, we show how to emphasize that light reflection, refraction and scattering can provide a proper, physical description of human perception of the "colour" white. These experiments can be used in the classroom with an enquiry…
Circularly symmetric light scattering from nanoplasmonic spirals.
Trevino, Jacob; Cao, Hui; Dal Negro, Luca
2011-05-11
In this paper, we combine experimental dark-field imaging, scattering, and fluorescence spectroscopy with rigorous electrodynamics calculations in order to investigate light scattering from planar arrays of Au nanoparticles arranged in aperiodic spirals with diffuse, circularly symmetric Fourier space. In particular, by studying the three main types of Vogel's spirals fabricated by electron-beam lithography on quartz substrates, we demonstrate polarization-insensitive planar light diffraction in the visible spectral range. Moreover, by combining dark-field imaging with analytical multiparticle calculations in the framework of the generalized Mie theory, we show that plasmonic spirals support distinctive structural resonances with circular symmetry carrying orbital angular momentum. The engineering of light scattering phenomena in deterministic structures with circular Fourier space provides a novel strategy for the realization of optical devices that fully leverage on enhanced, polarization-insensitive light-matter coupling over planar surfaces, such as thin-film plasmonic solar cells, plasmonic polarization devices, and optical biosensors.
Scattered light mapping of protoplanetary disks
Stolker, T.; Dominik, C.; Min, M.; Garufi, A.; Mulders, G. D.; Avenhaus, H.
2016-12-01
Context. High-contrast scattered light observations have revealed the surface morphology of several dozen protoplanetary disks at optical and near-infrared wavelengths. Inclined disks offer the opportunity to measure part of the phase function of the dust grains that reside in the disk surface which is essential for our understanding of protoplanetary dust properties and the early stages of planet formation. Aims: We aim to construct a method which takes into account how the flaring shape of the scattering surface of an optically thick protoplanetary disk projects onto the image plane of the observer. This allows us to map physical quantities (e.g., scattering radius and scattering angle) onto scattered light images and retrieve stellar irradiation corrected images (r2-scaled) and dust phase functions. Methods: The scattered light mapping method projects a power law shaped disk surface onto the detector plane after which the observed scattered light image is interpolated backward onto the disk surface. We apply the method on archival polarized intensity images of the protoplanetary disk around HD 100546 that were obtained with VLT/SPHERE in the R' band and VLT/NACO in the H and Ks bands. Results: The brightest side of the r2-scaled R' band polarized intensity image of HD 100546 changes from the far to the near side of the disk when a flaring instead of a geometrically flat disk surface is used for the r2-scaling. The decrease in polarized surface brightness in the scattering angle range of 40°-70° is likely a result of the dust phase function and degree of polarization which peak in different scattering angle regimes. The derived phase functions show part of a forward scattering peak, which indicates that large, aggregate dust grains dominate the scattering opacity in the disk surface. Conclusions: Projection effects of a protoplanetary disk surface need to be taken into account to correctly interpret scattered light images. Applying the correct scaling for the
Light Scattering Reviews, Vol 6 Light Scattering and Remote Sensing of Atmosphere and Surface
Kokhanovsky, Alexander A
2012-01-01
This is the next volume in series of Light Scattering Reviews. Volumes 1-5 have already been printed by Springer. The volume is composed of several papers ( usually, 10) of leading researchers in the respective field. The main focus of this book is light scattering, radiative transfer and optics of snow.
Lai, Puxiang; Tay, Jian Wei; Wang, Lihong V
2014-01-01
Non-invasively focusing light into strongly scattering media, such as biological tissue, is highly desirable but challenging. Recently, wavefront shaping technologies guided by ultrasonic encoding or photoacoustic sensing have been developed to address this limitation. So far, these methods provide only acoustic diffraction-limited optical focusing. Here, we introduce nonlinear photoacoustic wavefront shaping (PAWS), which achieves optical diffraction-limited (i.e. single-speckle-grain) focusing in scattering media. We develop an efficient dual-pulse excitation approach to generate strong nonlinear photoacoustic (PA) signals based on the Grueneisen memory effect. These nonlinear PA signals are used as feedback to guide iterative wavefront optimization. By maximizing the amplitude of the nonlinear PA signal, light is effectively focused to a single optical speckle grain. Experimental results demonstrate a clear optical focus on the scale of 5-7 micrometers, which is ~10 times smaller than the acoustic focus in...
High-Energy Compton Scattering Light Sources
Hartemann, Fred V; Barty, C; Crane, John; Gibson, David J; Hartouni, E P; Tremaine, Aaron M
2005-01-01
No monochromatic, high-brightness, tunable light sources currently exist above 100 keV. Important applications that would benefit from such new hard x-ray sources include: nuclear resonance fluorescence spectroscopy, time-resolved positron annihilation spectroscopy, and MeV flash radiography. The peak brightness of Compton scattering light sources is derived for head-on collisions and found to scale with the electron beam brightness and the drive laser pulse energy. This gamma 2
Pulsed Laser Nonlinear Thomson Scattering for General Scattering Geometries
Energy Technology Data Exchange (ETDEWEB)
Geoffrey Krafft; A. Doyuran; James Rosenzweig
2005-05-01
In a recent paper it has been shown that single electron Thomson backscatter calculations can be performed including the effects of pulsed high intensity lasers. In this paper we present a more detailed treatment of the problem and present results for more general scattering geometries. In particular, we present new results for 90 degree Thomson scattering. Such geometries have been increasingly studied as X-ray sources of short-pulse radiation. Also, we present a clearer physical basis for these different cases.
Light-like Scattering in Quantum Gravity
Bjerrum-Bohr, N E J; Holstein, Barry R; Plante, Ludovic; Vanhove, Pierre
2016-01-01
We consider scattering in quantum gravity and derive long-range classical and quantum contributions to the scattering of light-like bosons and fermions (spin-0, spin-1/2, spin-1) from an external massive scalar field, such as the Sun or a black hole. This is achieved by treating general relativity as an effective field theory and identifying the non-analytic pieces of the one-loop gravitational scattering amplitude. It is emphasized throughout the paper how modern amplitude techniques, involving spinor-helicity variables, unitarity, and squaring relations in gravity enable much simplified computations. We directly verify, as predicted by general relativity, that all classical effects in our computation are universal (in the context of matter type and statistics). Using an eikonal procedure we confirm the post-Newtonian general relativity correction for light-like bending around large stellar objects. We also comment on treating effects from quantum hbar dependent terms using the same eikonal method.
Light-like scattering in quantum gravity
Energy Technology Data Exchange (ETDEWEB)
Bjerrum-Bohr, N.E.J. [Niels Bohr International Academy & Discovery Center, Niels Bohr Institute,University of Copenhagen, Blegdamsvej 17, Copenhagen Ø, DK-2100 (Denmark); Donoghue, John F. [Department of Physics-LGRT, University of Massachusetts,Amherst, MA, 01003 (United States); Holstein, Barry R. [Department of Physics-LGRT, University of Massachusetts,Amherst, MA, 01003 (United States); Kavli Institute for Theoretical Physics, University of California,Santa Barbara, CA, 93016 (United States); Planté, Ludovic; Vanhove, Pierre [CEA, DSM, Institut de Physique Théorique, IPhT, CNRS MPPU, URA2306,Saclay, Gif-sur-Yvette, F-91191 (France)
2016-11-21
We consider scattering in quantum gravity and derive long-range classical and quantum contributions to the scattering of light-like bosons and fermions (spin-0, spin-(1/2), spin-1) from an external massive scalar field, such as the Sun or a black hole. This is achieved by treating general relativity as an effective field theory and identifying the non-analytic pieces of the one-loop gravitational scattering amplitude. It is emphasized throughout the paper how modern amplitude techniques, involving spinor-helicity variables, unitarity, and squaring relations in gravity enable much simplified computations. We directly verify, as predicted by general relativity, that all classical effects in our computation are universal (in the context of matter type and statistics). Using an eikonal procedure we confirm the post-Newtonian general relativity correction for light-like bending around large stellar objects. We also comment on treating effects from quantum ℏ dependent terms using the same eikonal method.
Light-like scattering in quantum gravity
Bjerrum-Bohr, N. E. J.; Donoghue, John F.; Holstein, Barry R.; Planté, Ludovic; Vanhove, Pierre
2016-11-01
We consider scattering in quantum gravity and derive long-range classical and quantum contributions to the scattering of light-like bosons and fermions (spin-0, spin- 1/2 , spin-1) from an external massive scalar field, such as the Sun or a black hole. This is achieved by treating general relativity as an effective field theory and identifying the non-analytic pieces of the one-loop gravitational scattering amplitude. It is emphasized throughout the paper how modern amplitude techniques, involving spinor-helicity variables, unitarity, and squaring relations in gravity enable much simplified computations. We directly verify, as predicted by general relativity, that all classical effects in our computation are universal (in the context of matter type and statistics). Using an eikonal procedure we confirm the post-Newtonian general relativity correction for light-like bending around large stellar objects. We also comment on treating effects from quantum ℏ dependent terms using the same eikonal method.
Protoplanetary disks and exoplanets in scattered light
Stolker, T.
2017-01-01
High-contrast imaging facilitates the direct detection of protoplanetary disks in scattered light and self-luminous exoplanets on long-period orbits. The combined power of extreme adaptive optics and differential imaging techniques delivers high spatial resolution images of disk morphologies down to
Nonlinear images of scatterers in chirped pulsed laser beams
Institute of Scientific and Technical Information of China (English)
Hu Yong-Hua; Wang You-Wen; Wen Shuang-Chun; Fan Dian-Yuan
2010-01-01
The bandwidth and the duration of incident pulsed beam are proved to play important roles in modifying the nonlinear image of amplitude-type scatterer.It is found that the initially positive chirp-type bandwidth can suppress the nonlinear image,while the negative one can enhance it,and that both effects are inversely proportional to the incident pulse duration.Numerical simulations further demonstrate that the location of nonlinear image is at the conjugate plane of the scatterer and that,for negatively pre-chirped pulsed beam,the nonlinear image peak intensity can be higher than that in the corresponding monochromatic case under certain conditions.Moreover the effect of group velocity dispersion on nonlinear image is found to be similar to that of chirp-type bandwidth.
A Recursive Born Approach to Nonlinear Inverse Scattering
Kamilov, Ulugbek S; Mansour, Hassan; Boufounos, Petros T
2016-01-01
The Iterative Born Approximation (IBA) is a well-known method for describing waves scattered by semi-transparent objects. In this paper, we present a novel nonlinear inverse scattering method that combines IBA with an edge-preserving total variation (TV) regularizer. The proposed method is obtained by relating iterations of IBA to layers of a feedforward neural network and developing a corresponding error backpropagation algorithm for efficiently estimating the permittivity of the object. Simulations illustrate that, by accounting for multiple scattering, the method successfully recovers the permittivity distribution where the traditional linear inverse scattering fails.
Scattered light mapping of protoplanetary disks
Stolker, T; Min, M; Garufi, A; Mulders, G D; Avenhaus, H
2016-01-01
High-contrast scattered light observations have revealed the surface morphology of several dozens of protoplanetary disks at optical and near-infrared wavelengths. Inclined disks offer the opportunity to measure part of the phase function of the dust grains that reside in the disk surface which is essential for our understanding of protoplanetary dust properties and the early stages of planet formation. We aim to construct a method which takes into account how the flaring shape of the scattering surface of an (optically thick) protoplanetary disk projects onto the image plane of the observer. This allows us to map physical quantities (scattering radius and scattering angle) onto scattered light images and retrieve stellar irradiation corrected (r^2-scaled) images and dust phase functions. We apply the method on archival polarized intensity images of the protoplanetary disk around HD 100546 that were obtained with VLT/SPHERE in R'-band and VLT/NACO in H- and Ks-band. The brightest side of the r^2-scaled R'-ban...
Light-shift-induced photonic nonlinearities
Energy Technology Data Exchange (ETDEWEB)
Brandao, F G S L; Hartmann, M J; Plenio, M B [Institute for Mathematical Sciences, Imperial College London, 53 Exhibition Road, SW7 2PE (United Kingdom)], E-mail: fernando@brandao@imperial.ac.uk
2008-04-15
We propose a new method to produce self- and cross-Kerr photonic nonlinearities, using light-induced Stark shifts due to the interaction of a cavity mode with atoms. The proposed experimental set-up is simpler than in previous approaches, while the strength of the nonlinearity obtained with a single atom is the same as in the setting based on electromagnetically induced transparency. Furthermore our scheme can be applied to engineer effective photonic nonlinear interactions whose strength increases with the number of atoms coupled to the cavity mode, leading to photon-photon interactions several orders of magnitude larger than previously considered possible.
Nonlinear single Compton scattering of an electron wave-packet
Angioi, A; Di Piazza, A
2016-01-01
In the presence of a sufficiently intense electromagnetic laser field, an electron can absorb on average a large number of photons from the laser and emit a high-energy one (nonlinear single Compton scattering). The case of nonlinear single Compton scattering by an electron with definite initial momentum has been thoroughly investigated in the literature. Here, we consider a more general initial state of the electron and use a wave-packet obtained as a superposition of Volkov wave functions. In particular, we investigate the energy spectrum of the emitted radiation at fixed observation direction and show that in typical experimental situations the sharply peaked structure of nonlinear single Compton scattering spectra of an electron with definite initial energy is almost completely washed out. Moreover, we show that at comparable uncertainties, the one in the momentum of the incoming electron has a larger impact on the photon spectra at a fixed observation direction than the one on the laser frequency, relate...
Nonlinear light propagation in chalcogenide photonic crystal slow light waveguides.
Suzuki, Keijiro; Baba, Toshihiko
2010-12-06
Optical nonlinearity can be enhanced by the combination of highly nonlinear chalcogenide glass and photonic crystal waveguides (PCWs) providing strong optical confinement and slow-light effects. In a Ag-As(2)Se(3) chalcogenide PCW, the effective nonlinear parameter γeff reaches 6.3 × 10(4) W(-1)m(-1), which is 200 times larger than that in Si photonic wire waveguides. In this paper, we report the detailed design, fabrication process, and the linear and nonlinear characteristics of this waveguide at silica fiber communication wavelengths. We show that the waveguide exhibits negligible two-photon absorption, and also high-efficiency self-phase modulation and four-wave mixing, which are assisted by low-dispersion slow light.
Light scattering studies of an electrorheological fluid
Energy Technology Data Exchange (ETDEWEB)
Martin, J.E.; Odinek, J.
1993-08-01
We report real-time, two-dimensional light scattering studies of the evolution of structure in an electrorheological fluid in the quiescent state and under shear. We find that when an electric field is applied to the quiescent fluid, particles chain along the electric field lines and cause strong light scattering lobes to appear at a finite scattering wavevector q orthogonal to the field lines. These lobes then brighten as they move to q=O, indicating the existence of an unstable concentration fluctuation that signifies the segregation of chains into columns. In fact, the observed power law growth kinetics of the characteristic length, as well as the form of the structure factor, are qualitatively similar to two-dimensional spinodal decomposition in a system with a conserved order parameter. When the sample is subjected to shear, we find that the scattering pattern approaches a steady state, with lobes that are rotated in the direction of fluid vorticity. The angle of rotation is found to increase as the cube root of the shear rate, in agreement with a theoretical prediction of the steady state structure of fragmenting particle chains.
Cooperativity in light scattering by cold atoms
Bienaime, Tom; Piovella, Nicola; Kaiser, Robin
2012-01-01
A cloud of cold N two-level atoms driven by a resonant laser beam shows cooperative effects both in the scattered radiation field and in the radiation pressure force acting on the cloud center-of-mass. The induced dipoles synchronize and the scattered light presents superradiant and/or subradiant features. We present a quantum description of the process in terms of a master equation for the atomic density matrix in the scalar, Born-Markov approximations, reduced to the single-excitation limit. From a perturbative approach for weak incident field, we derive from the master equation the effective Hamiltonian, valid in the linear regime. We discuss the validity of the driven timed Dicke ansatz and of a partial wave expansion for different optical thicknesses and we give analytical expressions for the scattered intensity and the radiation pressure force on the center of mass. We also derive an expression for collective suppression of the atomic excitation and the scattered light by these correlated dipoles.
Zeno: Critical Fluid Light Scattering Experiment
Gammon, Robert W.; Shaumeyer, J. N.; Briggs, Matthew E.; Boukari, Hacene; Gent, David A.; Wilkinson, R. Allen
1996-01-01
The Zeno (Critical Fluid Light Scattering) experiment is the culmination of a long history of critical fluid light scattering in liquid-vapor systems. The major limitation to making accurate measurements closer to the critical point was the density stratification which occurs in these extremely compressible fluids. Zeno was to determine the critical density fluctuation decay rates at a pair of supplementary angles in the temperature range 100 mK to 100 (mu)K from T(sub c) in a sample of xenon accurately loaded to the critical density. This paper gives some highlights from operating the instrument on two flights March, 1994 on STS-62 and February, 1996 on STS-75. More detail of the experiment Science Requirements, the personnel, apparatus, and results are displayed on the Web homepage at http://www.zeno.umd.edu.
Light scattering measurement of sodium polyacrylate products
Lama, Nisha; Norwood, David; Boone, Steven; Massie-Boyer, Valerie
2015-03-01
In the presentation, we will describe the use of a multi-detector HPLC incorporating the DAWN EOS multi-angle laser light scattering (MALLS) detector to measure the properties such as molecular weight, RMS radius, contour and persistence length and polydispersity of sodium polyacrylate products. The samples of sodium polyacrylate are used in various industries as thickening agents, coating dispersants, artificial snow, laundry detergent and disposable diapers. Data and results obtained from the experiment will be presented.
Characterization of Acryl amide Resins Using Static Light Scattering
Libi, Sumit; Norwood, David
2012-02-01
Our research is based on the use of light scattering technique for the characterization of known and unknown particles within a liquid. The research focused specifically on the detection of resin polymer that may be present in the given samples using static light scattering. The sample was delivered into a high performance liquid chromatography system with static light scattering, refractive index and viscosity detectors. Static Light scattering measures the intensity of the light scattered as the function of scattering angle and polymer sample concentration. Based on these results the molecular weight and radius of gyration of the given sample can be calculated.
Theory of diffusive light scattering cancellation cloaking
Farhat, Mohamed; Guenneau, Sebastien; Bagci, Hakan; Salama, Khaled Nabil; Alu, Andrea
2016-01-01
We report on a new concept of cloaking objects in diffusive light regime using the paradigm of the scattering cancellation and mantle cloaking techniques. We show numerically that an object can be made completely invisible to diffusive photon density waves, by tailoring the diffusivity constant of the spherical shell enclosing the object. This means that photons' flow outside the object and the cloak made of these spherical shells behaves as if the object were not present. Diffusive light invisibility may open new vistas in hiding hot spots in infrared thermography or tissue imaging.
Mid-infrared (λ = 8.4-9.9 μm) light scattering from porcine tissue
Liakat, Sabbir; Michel, Anna P. M.; Bors, Kevin A.; Gmachl, Claire F.
2012-08-01
Back-scattering of mid-infrared light from porcine skin is studied versus wavelength and angle for a Quantum Cascade laser and a broadband infrared light source. Scattering is detected over 30° away from the specular angle for both sources, and modulation patterns with angle are seen when using the laser. A nonlinear increase in scattered light intensity versus input power indicates that directional scattering from within the skin is dominant. Collagen fibers in the dermis layer, over 200 μm deep into the skin, are conducive to such scattering. We conclude that mid-infrared light penetrates deep enough for potential glucose detection in dermal interstitial fluid.
Scattering in the nonlinear Lamb system
Energy Technology Data Exchange (ETDEWEB)
Komech, A.I. [Faculty of Mathematics of Vienna University, Vienna (Austria); Institute for the Information Transmission Problems of RAS, Moscow (Russian Federation)], E-mail: alexander.komech@univie.ac.at; Merzon, A.E. [Institute of Physics and Mathematics, University of Michoacan of San Nicolas de Hidalgo, Morelia, Michoacan (Mexico)], E-mail: anatoli@ifm.imich.mx
2009-03-09
We obtain long time asymptotics for the solutions to a string coupled to a nonlinear oscillator: each finite energy solution decays to a sum of a stationary state and a dispersive wave. The asymptotics hold in global energy norm. The dispersive waves are expressed via initial data and solution to an ordinary differential equation. The asymptotics give a mathematical model for the Bohr's transitions between quantum stationary states.
Model of Light Scattering in Cavitation Area
Directory of Open Access Journals (Sweden)
S. P. Skvortsov
2015-01-01
Full Text Available The offered work presents analysis of extinction mechanisms and justification of light scattering model in ultrasonic cavitation area to justify a control method of ultrasonic cavitation through its optical sounding by low-intensity laser radiation and through photo-detector record of last radiation.The analysis of the extinction mechanisms has shown that the most essential mechanism causing a change of the transmission coefficient with time is dispersion on pulsating cavitation bubbles. Other extinction mechanisms lead to the time-constant reduction of last radiation intensity and can be taken into consideration by normalizing a recorded transmission coefficient for a previously measured liquid transmission coefficient when there is no cavitation.The feature of light scattering on the cavitation bubbles is primary dispersion in a forward direction that is connected with great values of bubbles radius from units to hundreds of micrometers. In case of single bubbles, dispersion can be described by Mi's theory, and, as to the cavitation area, it is reasonable to use the theory of V. Tversky for multiple light scattering. Thus, dispersion section, according to the paradox of extinction, can be considered to be equal to doubled geometrical section of a bubble. With increasing bubble radius the transmission coefficient monotonically decreases. So, the law of bubble pulsations and the model of light scattering define the law of changing transmission coefficient.Therefore, the cavitation area with its optical sounding acts as a peculiar opto-acoustic modulator. Thus, the demodulated signal of a photo-detector comprises information on pulsations of bubbles.The paper examines the influence of cavitation area thickness and bubbles concentration on the transmission coefficient. It shows a type of transmission coefficient dependence on the radius of cavitation bubbles.The optical sounding method is attractive because it allows us to obtain data on the
Measurements Of Scattered Light From Asbestos Particulate
Riis, P.; Ballik, E. A.
1987-09-01
Light-scattering techniques are potentially very important for the low-level detection and identification of particulate species such as asbestos in aerosol and liquid suspensions. Low-level detection is essential because asbestos is a known carcinogen, even at very-low exposure levels. At present, most asbestos particulate monitoring is used on optical microscopy. If detailed analysis is required, then electron microscopy is employed. Both of these methods are labour intensive. Furthermore, the optical microscopy method is not very reliable. Although the light-scattering techniques described here have general applicability, the emphasis is on asbestos measurements. Ordinary measurements of Mie scattering from asbestos suspensions can provide only limited information on asbestos content. owever, a more sophisticated technique can be employed which relies on the fact that asbestos particulate is fibrous rather than spherical in shape, and that the fibres align in a strong magnetic field (approximately 0.5 T). Particulate other than asbestos is generally non-fibrous in shape. Measurements have been carried out on liquid suspensions of asbestos contained in a small cell placed between the poles of a rotating magnet. The aligned fibres, which rotate about their centre of mass as they follow the field, are illuminated using a laser source. The Mie-scattering intensity is measured as a function of rotation angle, and the resulting data is then analysed with the aid of a microcomputer. Intensity maxima and minima provide reliable information on asbestos concentration, even in the presence of strong scattering from other particulate. In addition, the angular location of the intensity peaks provides information on the type of asbestos present. Each type has a characteristic alignment behaviour in a strong magnetic field. Using relatively-simple equipment, chrysotile asbestos (the most commonly-used type) has been detected at levels below 30 ng/l.
Energy Technology Data Exchange (ETDEWEB)
Artemyev, A. V., E-mail: ante0226@gmail.com; Vasiliev, A. A. [Space Research Institute, RAS, Moscow (Russian Federation); Mourenas, D.; Krasnoselskikh, V. V. [LPC2E/CNRS—University of Orleans, Orleans (France); Agapitov, O. V. [Space Sciences Laboratory, University of California, Berkeley, California 94720 (United States)
2014-10-15
In this paper, we consider high-energy electron scattering and nonlinear trapping by oblique whistler waves via the Landau resonance. We use recent spacecraft observations in the radiation belts to construct the whistler wave model. The main purpose of the paper is to provide an estimate of the critical wave amplitude for which the nonlinear wave-particle resonant interaction becomes more important than particle scattering. To this aim, we derive an analytical expression describing the particle scattering by large amplitude whistler waves and compare the corresponding effect with the nonlinear particle acceleration due to trapping. The latter is much more rare but the corresponding change of energy is substantially larger than energy jumps due to scattering. We show that for reasonable wave amplitudes ∼10–100 mV/m of strong whistlers, the nonlinear effects are more important than the linear and nonlinear scattering for electrons with energies ∼10–50 keV. We test the dependencies of the critical wave amplitude on system parameters (background plasma density, wave frequency, etc.). We discuss the role of obtained results for the theoretical description of the nonlinear wave amplification in radiation belts.
ATLAS Event Display: Light-by-Light Scattering
ATLAS Collaboration
2017-01-01
An event display of light-by-light scattering in ultra-peripheral lead+lead collisions at 5.02 TeV with the ATLAS detector at the LHC. The event 461251458 from run 287931 recorded on 13 December 2015 at 09:51:07 is shown. Two back-to-back photons with an invariant mass of 24 GeV with no additional activity in the detector are presented. All calorimeter cells with E>500 MeV are shown.
arXiv Light-by-Light Scattering Constraint on Born-Infeld Theory
Ellis, John; You, Tevong
2017-06-27
The recent measurement by ATLAS of light-by-light scattering in LHC Pb-Pb collisions is the first direct evidence for this basic process. We find that it excludes a range of the mass scale of a nonlinear Born-Infeld extension of QED that is ≲100 GeV, a much stronger constraint than those derived previously. In the case of a Born-Infeld extension of the standard model in which the U(1)Y hypercharge gauge symmetry is realized nonlinearly, the limit on the corresponding mass reach is ∼90 GeV, which, in turn, imposes a lower limit of ≳11 TeV on the magnetic monopole mass in such a U(1)Y Born-Infeld theory.
Nonlinear optics with stationary pulses of light
Andre, A.; Bajcsy, M.; Zibrov, A. S.; Lukin, M. D.
2004-01-01
We show that the recently demonstrated technique for generating stationary pulses of light [Nature {\\bf 426}, 638 (2003)] can be extended to localize optical pulses in all three spatial dimensions in a resonant atomic medium. This method can be used to dramatically enhance the nonlinear interaction between weak optical pulses. In particular, we show that an efficient Kerr-like interaction between two pulses can be implemented as a sequence of several purely linear optical processes. The resul...
Nonlinear scattering of radio waves by metal objects
Shteynshleyger, V. B.
1984-07-01
Nonlinear scattering of radio waves by metal structures with resulting harmonic and intermodulation interference is analyzed from both theoretical and empirical standpoints, disregarding nonlinear effects associated with the nonlinear dependence of the electric or magnetic polarization vector on respectively the electric or magnetic field intensity in the wave propagating medium. Nonlinear characteristics of metal-oxide-metal contacts where the thin oxide film separation two metal surfaces has properties approximately those of a dielectric or a high-resistivity semiconductor are discussed. Tunneling was found to be the principal mechanism of charge carrier transfer through such a contact with a sufficiently thin film, the contact having usually a cubic or sometimes an integral sign current-voltage characteristic at 300 K and usually S-form or sometimes a cubic current-voltage characteristic at 77 K.
Nonreciprocal wave scattering on nonlinear string-coupled oscillators
Energy Technology Data Exchange (ETDEWEB)
Lepri, Stefano, E-mail: stefano.lepri@isc.cnr.it [Consiglio Nazionale delle Ricerche, Istituto dei Sistemi Complessi, via Madonna del Piano 10, I-50019 Sesto Fiorentino (Italy); Istituto Nazionale di Fisica Nucleare, Sezione di Firenze, via G. Sansone 1, I-50019 Sesto Fiorentino (Italy); Pikovsky, Arkady [Department of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str 24/25, Potsdam (Germany); Department of Control Theory, Nizhni Novgorod State University, Gagarin Av. 23, 606950, Nizhni Novgorod (Russian Federation)
2014-12-01
We study scattering of a periodic wave in a string on two lumped oscillators attached to it. The equations can be represented as a driven (by the incident wave) dissipative (due to radiation losses) system of delay differential equations of neutral type. Nonlinearity of oscillators makes the scattering non-reciprocal: The same wave is transmitted differently in two directions. Periodic regimes of scattering are analyzed approximately, using amplitude equation approach. We show that this setup can act as a nonreciprocal modulator via Hopf bifurcations of the steady solutions. Numerical simulations of the full system reveal nontrivial regimes of quasiperiodic and chaotic scattering. Moreover, a regime of a “chaotic diode,” where transmission is periodic in one direction and chaotic in the opposite one, is reported.
Noninvasive nonlinear imaging through strongly-scattering turbid layers
Katz, Ori; Guan, Yefeng; Silberberg, Yaron
2014-01-01
Diffraction-limited imaging through complex scattering media is a long sought after goal with important applications in biomedical research. In recent years, high resolution wavefront-shaping has emerged as a powerful approach to generate a sharp focus through highly scattering, visually opaque samples. However, it requires a localized feedback signal from the target point of interest, which necessitates an invasive procedure in all-optical techniques. Here, we show that by exploiting optical nonlinearities, a diffraction-limited focus can be formed inside or through a complex sample, even when the feedback signal is not localized. We prove our approach theoretically and numerically, and experimentally demonstrate it with a two-photon fluorescence signal through highly scattering biological samples. We use the formed focus to perform two-photon microscopy through highly scattering, visually opaque layers.
Industrial Particle Size Measurement Using Light Scattering
Muly, E. C.; Frock, H. N.
1980-12-01
The precise knowledge of particle size and particle size distribution is fundamental to the control of a wide variety of industrial processes. Processing steps as diverse as crystallization, grinding, emulsification, and atomization, produce particles in the size range .1 to 1000 micrometers in diameter. While the object of some processes may be the production of particles of specified sizes, e.g., abrasives and glass beads, other processes may require particle size control for process efficiency, e.g., crystallization, and still others for control of final product quality, e.g., minerals, cement, and ceramics. In many processes more than one of these reasons may be important. A line of instruments has been developed using light scattering to measure various parameters of particulate distributions. These instruments employ laser illumination of a flowing stream of particles, producing Fraunhofer diffraction patterns which are processed both optically and electronically with unique, proprietary techniques. Various parameters of the particle size distribution are measured. The measurement is both rapid and precise. This paper will cover the importance of particle size measurements in various processes, different types of measurement methods, and the application of light scattering technology to size determinations in wet slurries and dry powders. A number of specific applications will be discussed encompassing minerals grinding, Portland cement, and rolling mill emulsions. Some references will be made to energy savings through automation.
Fourier transform light scattering angular spectroscopy using digital inline holography.
Kim, Kyoohyun; Park, YongKeun
2012-10-01
A simple and practical method for measuring the angle-resolved light scattering (ARLS) from individual objects is reported. Employing the principle of inline holography and a Fourier transform light scattering technique, both the static and dynamic scattering patterns from individual micrometer-sized objects can be effectively and quantitatively obtained. First, the light scattering measurements were performed on individual polystyrene beads, from which the refractive index and diameter of each bead were retrieved. Also, the measurements of the static and dynamic light scattering from intact human red blood cells are demonstrated. Using the present method, an existing microscope can be directly transformed into a precise instrument for ARLS measurements.
Institute of Scientific and Technical Information of China (English)
胡业民; 胡希伟
2001-01-01
Numerical analyses for the nonlinear evolutions of stimulated Raman scattering (SRS) and stimulated Brillouin scattering (SBS) processes are given. Various effects of the second- and third-order nonlinear susceptibilities on the SRS and SBS processes are studied. The nonlinear evolutions of SRS and SBS processes are atfected more efficiently than their linear growth rates by the nonlinear susceptibility.
Rayleigh scattering and nonlinear inversion of elastic waves
Energy Technology Data Exchange (ETDEWEB)
Gritto, R.
1995-12-01
Rayleigh scattering of elastic waves by an inclusion is investigated and the limitations determined. In the near field of the inhomogeneity, the scattered waves are up to a factor of 300 stronger than in the far field, excluding the application of the far field Rayleigh approximation for this range. The investigation of the relative error as a function of parameter perturbation shows a range of applicability broader than previously assumed, with errors of 37% and 17% for perturbations of {minus}100% and +100%, respectively. The validity range for the Rayleigh limit is controlled by large inequalities, and therefore, the exact limit is determined as a function of various parameter configurations, resulting in surprisingly high values of up to k{sub p}R = 0.9. The nonlinear scattering problem can be solved by inverting for equivalent source terms (moments) of the scatterer, before the elastic parameters are determined. The nonlinear dependence between the moments and the elastic parameters reveals a strong asymmetry around the origin, which will produce different results for weak scattering approximations depending on the sign of the anomaly. Numerical modeling of cross hole situations shows that near field terms are important to yield correct estimates of the inhomogeneities in the vicinity of the receivers, while a few well positioned sources and receivers considerably increase the angular coverage, and thus the model resolution of the inversion parameters. The pattern of scattered energy by an inhomogeneity is complicated and varies depending on the object, the wavelength of the incident wave, and the elastic parameters involved. Therefore, it is necessary to investigate the direction of scattered amplitudes to determine the best survey geometry.
Discrimination of airborne material particles from light scattering (TAOS) patterns
Crosta, Giovanni F.; Pan, Yong-Le; Videen, Gorden; Aptowicz, Kevin B.; Chang, Richard K.
2013-05-01
Two-dimensional angle-resolved optical scattering (TAOS) is an experimental method which collects the intensity pattern of monochromatic light scattered by a single, micron-sized airborne particle. In general, the interpretation of these patterns and the retrieval of the particle refractive index, shape or size alone, are difficult problems. The solution proposed herewith relies on a learning machine (LM): rather than identifying airborne particles from their scattering patterns, TAOS patterns themselves are classified. The LM consists of two interacting modules: a feature extraction module and a linear classifier. Feature extraction relies on spectrum enhancement, which includes the discrete cosine Fourier transform and non-linear operations. Linear classification relies on multivariate statistical analysis. Interaction enables supervised training of the LM. The application described in this article aims at discriminating the TAOS patterns of single bacterial spores (Bacillus subtilis) from patterns of atmospheric aerosol and diesel soot particles. The latter are known to interfere with the detection of bacterial spores. Classification has been applied to a data set with more than 3000 TAOS patterns from various materials. Some classification experiments are described, where the size of training sets has been varied as well as many other parameters which control the classifier. By assuming all training and recognition patterns to come from the respective reference materials only, the most satisfactory classification result corresponds to ≍ 20% false negatives from Bacillus subtilis particles and <= 11% false positives from environmental and diesel particles.
Extinction and Scattering of Light by Magnetic Colloidal Nanoparticles
Directory of Open Access Journals (Sweden)
C.V. Yerin
2015-12-01
Full Text Available The peculiarities of scattering and extinction of light by colloids with different concentrations of magnetite nanoparticles are investigated. The light absorption effect on spectral dependencies of optical density of magnetic colloid are observed. According to dynamic light scattering experiments, particle size distributions for samples with different concentration of nanoparticles are defined.
Energy Technology Data Exchange (ETDEWEB)
Walker, Bennett N., E-mail: bennett.walker@fda.hhs.gov [Optical Therapeutics and Medical Nanophotonics Laboratory, Office of Science and Engineering Laboratories, U.S. Food and Drug Administration, Silver Spring, Maryland 20993 (United States); Office of Device Evaluation, Center for Devices and Radiological Health, U.S. Food and Drug Administration, Silver Spring, Maryland 20993 (United States); James, Robert H.; Ilev, Ilko K. [Optical Therapeutics and Medical Nanophotonics Laboratory, Office of Science and Engineering Laboratories, U.S. Food and Drug Administration, Silver Spring, Maryland 20993 (United States); Calogero, Don [Office of Device Evaluation, Center for Devices and Radiological Health, U.S. Food and Drug Administration, Silver Spring, Maryland 20993 (United States)
2015-09-15
Glare, glistenings, optical defects, dysphotopsia, and poor image quality are a few of the known deficiencies of intraocular lenses (IOLs). All of these optical phenomena are related to light scatter. However, the specific direction that light scatters makes a critical difference between debilitating glare and a slightly noticeable decrease in image quality. Consequently, quantifying the magnitude and direction of scattered light is essential to appropriately evaluate the safety and efficacy of IOLs. In this study, we introduce a full-angle scanning light scattering profiler (SLSP) as a novel approach capable of quantitatively evaluating the light scattering from IOLs with a nearly 360° view. The SLSP method can simulate in situ conditions by controlling the parameters of the light source including angle of incidence. This testing strategy will provide a more effective nonclinical approach for the evaluation of IOL light scatter.
Measurement of Dynamic Light Scattering Intensity in Gels
Rochas, Cyrille
2015-01-01
In the scientific literature little attention has been given to the use of dynamic light scattering (DLS) as a tool for extracting the thermodynamic information contained in the absolute intensity of light scattered by gels. In this article we show that DLS yields reliable measurements of the intensity of light scattered by the thermodynamic fluctuations, not only in aqueous polymer solutions, but also in hydrogels. In hydrogels, light scattered by osmotic fluctuations is heterodyned by that from static or slowly varying inhomogeneities. The two components are separable owing to their different time scales, giving good experimental agreement with macroscopic measurements of the osmotic pressure. DLS measurements in gels are, however, tributary to depolarised light scattering from the network as well as to multiple light scattering. The paper examines these effects, as well as the instrumental corrections required to determine the osmotic modulus. For guest polymers trapped in a hydrogel the measured intensity...
How to distinguish elastically scattered light from Stokes shifted light for solid-state lighting?
Meretska, M. L.; Lagendijk, A.; Thyrrestrup, H.; Mosk, A. P.; IJzerman, W. L.; Vos, W.L.
2016-01-01
We have studied the transport of light through phosphor diff user plates that are used in commercial solid-state lighting modules (Fortimo). These polymer plates contain YAG:Ce+3 phosphor particles that both elastically scatter and Stokes shift light in the visible wavelength range (400-700 nm). We
Miniature instrumentation for laser light scattering experiments
Brown, Robert G. W.
1989-01-01
Traditional optical systems for photon correlation spectroscopy and laser anemometry have relied upon physically large and fairly expensive lasers, bulk-optics such as lenses of a few inches diameter, large mechanical mounts and carefully selected, fragile and bulky photon counting photomultiplier detectors. In some cases, experimental fluid dynamics at a desired position in a flow, perhaps deep inside complex machinery, is physically impossible or very difficult. Similar problems exist with photon correlation spectroscopy, e.g., remote and heterodyne experiments. Various optical and electro optical components were investigated and characterized with the aim of replacing existing photon correlation laser spectroscopy and anemometry techniques in miniaturized form, and with significant cost reduction. Very recently, a range of miniature, modular light scattering systems were constructed from little solid state optical and electro optical components, and experimentally verified measurement performance comparable to standard lab photon correlation spectroscopy and laser anemometry equipment.
Scattering of light by charged colloidal particles in salt solutions
Vrij, A.; Overbeek, J.Th.G.
1962-01-01
In the interpretation of light scattering by colloidal electrolytes in salt solutions the interaction between the colloidal particles and the low molecular weight ions has to be taken into account. When fluctuation theory is applied for the derivation of a light-scattering equation, nonelectroneutra
Utility of light scatter in the morphological analysis of sperm
We were able to differentiate the morphologically diverse sperm nuclei of four animal species by using an Ortho flow cytometer to detect the forward light scatter from a red (helium-neon) laser. Cytograms depicting the axial light loss and forward red scatter signals revealed uni...
Light scattering by neutrophils: Model, simulation, and experiment
Orlova, D.Y.; Yurkin, M.A.; Hoekstra, A.G.; Maltsev, V.P.
2008-01-01
We studied the elastic light-scattering properties of human blood neutrophils, both experimentally and theoretically. The experimental study was performed with a scanning flow cytometer measuring the light-scattering patterns (LSPs) of individual cells over an angular range of 5-60 deg. We determine
Nonlinear double Compton scattering in the full quantum regime
Mackenroth, F
2012-01-01
A detailed analysis of the process of two photon emission by an electron scattered from a high-intensity laser pulse is presented. The calculations are performed in the framework of strong-field QED and include exactly the presence of the laser field, described as a plane wave. We investigate the full quantum regime of interaction, where photon recoil plays an essential role in the emission process, and substantially alters the emitted photon spectra as compared to those in previously-studied regimes. We provide a semiclassical explanation for such differences, based on the possibility of assigning a trajectory to the electron in the laser field before and after each quantum photon emission. Our numerical results indicate the feasibility of investigating experimentally the full quantum regime of nonlinear double Compton scattering with already available plasma-based electron accelerator and laser technology.
Light scattering by marine heterotrophic bacteria
Ulloa, Osvaldo; Sathyendranath, Shubha; Platt, Trevor; Quinones, Renato A.
1992-01-01
Mie theory is applied to estimate scattering by polydispersions of marine heterotrophic bacteria, and a simple expression is derived for the bacterial scattering coefficient. The error incurred in deriving bacterial optical properties by use of the van de Hulst approximations is computed. The scattering properties of natural bacterial assemblages in three marine environments, Georges Bank, Northeast Channel, and Sargasso Sea, are assessed by applying Mie theory to field data on bacterial size and abundance. Results are used to examine the potential contribution of bacteria to the scattering properties of seawater. The utility of using pigment data to predict the magnitude of scattering by bacteria is discussed.
Improved algorithm of light scattering by a coated sphere
Institute of Scientific and Technical Information of China (English)
Lei Liu; Huarui Wang; Bin Yu; Yamin Xu; Jianqi Shen
2007-01-01
An efficient numerical algorithm for computing the light scattering by a coated sphere is proposed. The calculation of relevant functions by different recurrence algorithms is discussed. The new algorithm avoids the numerical difficulties, which give rise to significant errors encountered in practice by prior methods. Exemplifying results such as extinction efficiency, scattering efficiency, light scattering intensity as well as calculation speed are provided. The results show that this algorithm is efficient, fast, numerically stable and accurate.
Scattering of light by a system of anisotropic particles.
Du, Xinyue; Zhao, Daomu
2010-05-15
The cross-spectral density function of the scattered field that is produced by scattering of a coherent plane light wave incident on a collection of different types of anisotropic particles is derived. We show the phenomena of interference of the fields scattered by each of the particles in the system. Numerical results indicate that the information about the shape, the distance, and the relative orientation of the particles may be obtained from far-zone measurements of the scattered field.
Peak intensity measurement of relativistic lasers via nonlinear Thomson scattering
Har-Shemesh, Omri
2011-01-01
The measurement of peak laser intensities exceeding $10^{20}\\;\\text{W/cm$^2$}$ is in general a very challenging task. We suggest a simple method to accurately measure such high intensities up to about $10^{23}\\,\\text{W/cm$^2$}$, by colliding a beam of ultrarelativistic electrons with the laser pulse. The method exploits the specific features of the angular distribution of the radiation emitted by ultrarelativistic electrons via nonlinear Thomson scattering. Initial electron energies well within the reach of laser wake-field accelerators are required, allowing in principle for an all-optical setup. Accuracies of the order of 10% are envisaged.
Macrovoids formation and light scattering of PMMA
Indian Academy of Sciences (India)
Zhi Hong Chen; Z C Chang; C B Lin
2007-08-01
After desorption of PMMA with saturated methanol and ethanol and then desorption by distilled water, the macrovoids are formed because of the phase inversion. The macrovoids on the surface of the specimens are larger and more numerous than those in the bulk. The macrovoids are likely to be closed-type, if the hydrolysis temperature is lower. On the other hand, if the hydrolysis temperature is higher, the macrovoids are likely to be open-type. Due to the formation of macrovoids, smaller than visible wavelengths, the light will disperse, and therefore, reduces the transmittance of the specimens. The transmittance is decreased when the hydrolysis temperature and hydrolysis time are increased. Furthermore, it is much clearer when ethanol is used as solvent than methanol. The scattered intensity of the specimens after hydrolysis is inversely proportional to the visible wavelength with an exponent, , in the range 0.04–2.83 for methanol and 0.02–0.21 for ethanol.
Light scattering of thin azobenzene side-chain polyester layers
DEFF Research Database (Denmark)
Kerekes, Á.; Lörincz, E.; Ramanujam, P.S.
2002-01-01
characteristics than the liquid crystalline polyester. The amorphous samples have negligible polarization part orthogonal to the incident beam. the liquid crystalline samples have relative high orthogonal polarization part in light scattering, The light scattering results can be used to give a lower limit...... for the domain size in thin liquid crystalline polyester layers being responsible for the dominant light scattering. The characteristic domain Sizes obtained from the Fourier transformation of polarization microscopic Pictures confirm these values.......Light scattering properties of liquid crystalline and amorphous azobenzene side-chain polyester layers used for optical data storage were examined by means of transmissive scatterometry. Comparative experiments show that the amorphous polyester has significantly lower light scattering...
Study of erythrocyte membrane fluctuation using light scattering analysis
Lee, Hoyoon; Lee, Sangyun; Park, YongKeun; Shin, Sehyun
2016-03-01
It is commonly known that alteration of erythrocyte deformability lead to serious microcirculatory diseases such as retinopathy, nephropathy, etc. Various methods and technologies have been developed to diagnose such membrane properties of erythrocytes. In this study, we developed an innovative method to measure hemorheological characteristics of the erythrocyte membrane using a light scattering analysis with simplified optic setting and multi-cell analysis as well. Light scattering intensity through multiple erythrocytes and its power density spectrum were obtained. The results of light scattering analyses were compared in healthy control and artificially hardened sample which was treated with glutaraldehyde. These results were further compared with conventional assays to measure deformable property in hemorheology. We found that light scattering information would reflect the disturbance of membrane fluctuation in artificially damaged erythrocytes. Therefore, measuring fluctuation of erythrocyte membrane using light scattering signal could facilitate simple and precise diagnose of pathological state on erythrocyte as well as related complications.
Positron Production in Multiphoton Light-by-Light Scattering
Energy Technology Data Exchange (ETDEWEB)
Koffas, Thomas
2003-07-28
We present the results of an experimental study on e{sup +}e{sup -} pair production during the collision of a low emittance 46.6 GeV electron beam with terawatt laser pulses from a Nd:glass laser at 527 nm wavelength and with linear polarization. The experiment was conducted at the Final Focus Test Beam facility in the Stanford Linear Accelerator Center. Results with a 49.1 GeV electron beam are also included. A signal of 106 {+-} 14 positrons for the 46.6 GeV electron beam case and of 22 {+-} 10 positrons for the 49.1 GcV case above background, has been detected. We interpret the positrons as the products of a two-step process during which laser photons are backscattered to high energy gamma photons that absorb in their turn several laser photons in order to produce a e{sup +}e{sup -} pair. The data compare well with the existing theoretical models. This is the first observation in the laboratory of inelastic Light-by-Light scattering with only real photons. Alternatively, the data are interpreted as a manifestation of the spontaneous breakdown of the vacuum under the influence of an intense external alternating electric field.
Andreev, A A; Zhidkov, A G; Uesaka, M; Kinoshita, K; Platonov, K Yu
2002-09-01
The light scattered backward from a target illuminated by ultraintense laser pulses carries important information about the nonlinear laser-plasma interaction. We analyze the usefulness of this information by plasma corona analysis with the help of an analytical model we developed, and particle-in-cell simulation. The spectrum of scattered light is shown to be shifted, to be broadened, and to be modulated, in comparison with the initial laser spectrum, and the spectral shift is an indicator of laser pulse contrast ratio.
Multiangle static and dynamic light scattering in the intermediate scattering angle range
Tamborini, Elisa
2012-01-01
We describe a light scattering apparatus based on a novel optical scheme covering the scattering angle range $0.5\\dg \\le \\theta \\le 25\\dg$, an intermediate regime at the frontier between wide angle and small angle setups that is difficult to access by existing instruments. Our apparatus uses standard, readily available optomechanical components. Thanks to the use of a charge-coupled device detector, both static and dynamic light scattering can be performed simultaneously at several scattering angles. We demonstrate the capabilities of our apparatus by measuring the scattering profile of a variety of samples and the Brownian dynamics of a dilute colloidal suspension.
Light scattering in Baltic crude oil - seawater emulsion
Directory of Open Access Journals (Sweden)
Adam Stelmaszewski
2009-09-01
Full Text Available The paper discusses the scattering of radiation by a Baltic crude oil - seawater emulsion. The scattering spectrum calculated using the Mie solution in the spectral range from 380 nm to 730 nm is compared with the measured spectrum of light scattered through a right angle. Spectra in the wavelength range from 210 nm to 730 nm were measured using a spectrofluorimeter for fresh and stored samples of the Baltic crude oil emulsion. Scattering increases with wavelength in the UV range and then decreases slightly with the wavelength of visible light. The result of the calculation is similar to the measured spectra. Both the calculated and measured spectra display numerous relative extremes throughout the spectral area. Light scattering in the emulsion decreases during storage as the oil concentration in the medium diminishes. The results also demonstrate that the single scattering model describes the phenomenon correctly.
Effects of cellular fine structure on scattered light pattern.
Liu, Caigen; Capjack, Clarence E
2006-06-01
Biological cells are complex in both morphological and biochemical structure. The effects of cellular fine structure on light scattered from cells are studied by employing a three-dimensional code named AETHER which solves the full set of Maxwell equations by using the finite-difference time-domain method. It is shown that changes in cellular fine structure can cause significant changes in the scattered light pattern over particular scattering angles. These changes potentially provide the possibility for distinguishability of cellular intrastructures. The effects that features of different intrastructure have on scattered light are discussed from the viewpoint of diagnosing cellular fine structure. Finally, we discuss scattered light patterns for lymphocyte-like cells and basophil-like cells.
Nonlinear Gain Saturation in Active Slow Light Photonic Crystal Waveguides
DEFF Research Database (Denmark)
Chen, Yaohui; Mørk, Jesper
2013-01-01
We present a quantitative three-dimensional analysis of slow-light enhanced traveling wave amplification in an active semiconductor photonic crystal waveguides. The impact of slow-light propagation on the nonlinear gain saturation of the device is investigated.......We present a quantitative three-dimensional analysis of slow-light enhanced traveling wave amplification in an active semiconductor photonic crystal waveguides. The impact of slow-light propagation on the nonlinear gain saturation of the device is investigated....
Sakata, Yoshitaro; Terasaki, Nao; Sakai, Kazufumi; Nonaka, Kazuhiro
2016-11-01
The stress-induced light scattering method (SILSM) was proposed for inspecting surface to detect polishing induced latent flaws. In this study, in order to clarify the mechanism of the light scattering intensity variation of latent flaws using SILSM, we have investigated stress effect of light scattering intensities using polarized light system and calculated the reflectance and the retardation using Jones matrix. As the results, we evaluated the change in the birefringence around a tip of a latent flaw between before and after stress were applied.
Absorption and scattering of light by small particles
Bohren, Craig F
1983-01-01
Absorption and Scattering of Light by Small Particles. Treating absorption and scattering in equal measure, this self-contained, interdisciplinary study examines and illustrates how small particles absorb and scatter light. The authors emphasize that any discussion of the optical behavior of small particles is inseparable from a full understanding of the optical behavior of the parent material-bulk matter. To divorce one concept from the other is to render any study on scattering theory seriously incomplete. Special features and important topics covered in this book include:. * Classical theor
Light scattering by nonspherical particles theory, measurements, and applications
Mishchenko, Michael I; Travis, Larry D
1999-01-01
There is hardly a field of science or engineering that does not have some interest in light scattering by small particles. For example, this subject is important to climatology because the energy budget for the Earth's atmosphere is strongly affected by scattering of solar radiation by cloud and aerosol particles, and the whole discipline of remote sensing relies largely on analyzing the parameters of radiation scattered by aerosols, clouds, and precipitation. The scattering of light by spherical particles can be easily computed using the conventional Mie theory. However, most small solid part
Correlating the morphological and light scattering properties of biological cells
Moran, Marina
The scattered light pattern from a biological cell is greatly influenced by the internal structure and optical properties of the cell. This research project examines the relationships between the morphological and scattering properties of biological cells through numerical simulations. The mains goals are: (1) to develop a procedure to analytically model biological cells, (2) to quantitatively study the effects of a range of cell characteristics on the features of the light scattering patterns, and (3) to classify cells based on the features of their light scattering patterns. A procedure to create an analytical cell model was developed which extracted structural information from the confocal microscopic images of cells and allowed for the alteration of the cell structure in a controlled and systematic way. The influence of cell surface roughness, nuclear size, and mitochondrial volume density, spatial distribution, size and shape on the light scattering patterns was studied through numerical simulations of light scattering using the Discrete Dipole Approximation. It was found that the light scattering intensity in the scattering angle range of 25° to 45° responded to changes in the surface fluctuation of the cell and the range of 90° to 110° was well suited for characterization of mitochondrial density and nuclear size. A comparison of light scattering pattern analysis methods revealed that the angular distribution of the scattered light and Gabor filters were most helpful in differentiating between the cell characteristics. In addition, a measured increase in the Gabor energy of the light scattering patterns in response to an increase in the complexity of the cell models suggested that a complex nuclear structure and mitochondria should be included when modeling biological cells for light scattering simulations. Analysis of the scattering pattern features with Gabor filters resulted in discrimination of the cell models according to cell surface roughness
Simulations of light-light scattering in quantum vacuum
Carneiro, Pedro; Grismayer, Thomas; Silva, LuíS.; Fonseca, Ricardo
2016-10-01
Facilities such as the Extreme Light Infrastructure (ELI) or the VULCAN 20 PW project, as well as the Petta-Watt SLAC project, coupled with the x-ray LCLSII source will allow to perform the first experiments on the probing of quantum vacuum. In our work, we developed a numerical method to self-consistently solve the nonlinear system of Maxwell's equations including quantum corrections of vacuum polarization. The robustness of our algorithm allied to the ability to integrate this tool within a particle-in-cell (PIC) method, represents an important milestone in modeling future planned experiments to prove the existence of the quantum vacuum. Such experiments aim to measure the induced ellipticity on a x-ray pulse after probing a strong optical pump due to the quantum vacuum fluctuations. We present simulation results of both the ellipticity induced and polarization rotation, using realistic laser parameters of the Petta-Watt SLAC project, and the x-ray LCLSII source, whilst taking into account all finite-size multi-dimensional effects. We show how the ellipticity induced varies as a function of the distance to the axis of the beam, proving the importance of taking into account finite-size effects. This work serves as an important tool to complement existing efforts within the community to probe the effects of the quantum vacuum, in the strong field regime, for the first time.
Light scattering by particles in water theoretical and experimental foundations
Jonasz, Miroslaw
2007-01-01
Light scattering-based methods are used to characterize small particles suspended in water in a wide range of disciplines ranging from oceanography, through medicine, to industry. The scope and accuracy of these methods steadily increases with the progress in light scattering research. This book focuses on the theoretical and experimental foundations of the study and modeling of light scattering by particles in water and critically evaluates the key constraints of light scattering models. It begins with a brief review of the relevant theoretical fundamentals of the interaction of light with condensed matter, followed by an extended discussion of the basic optical properties of pure water and seawater and the physical principles that explain them. The book continues with a discussion of key optical features of the pure water/seawater and the most common components of natural waters. In order to clarify and put in focus some of the basic physical principles and most important features of the experimental data o...
Measurements and interpretations of light scattering from intact biological cells
Wilson, Jeremy D.
Visible light interacts with biological cells primarily through elastic scattering. The details of how cells scatter light depend on their morphology and their substructures. In this thesis we first present a series of experiments and models to discern the specific contributions of certain sub-cellular constituents to whole-cell scattering. Exploiting the findings of those studies, we report on experiments within model systems of cell death that demonstrate the potential of light scattering measurements as a tool in modern biology. Instrumentation capable of exploiting the findings of this thesis from a biology-relevant microscopy platform is designed and developed. A Mie theory based interpretation of light scattering signals originating from a collection of particles with a broad size distribution is developed. Upon applying this model to scattering data from intact cells, we find that it robustly extracts the size scale of dominant light scattering particles, suggests that scattering measurements are sensitive primarily to mitochondrial and lysosomal morphology, and unites conflicting results in the literature. Using this model as a basis, we present a collection of studies in which we use various strategies of photodynamic therapy (PDT) as a biophysical tool to perturb mitochondria and lysosomes, and observe the effects of these perturbations on whole-cell scattering. Through these experiments, we are able to discern the individual contributions of mitochondria and lysosomes to whole-cell light scattering, and demonstrate that mitochondria are responsible for roughly 80% of the scattering signal. Results of experiments aimed at demonstrating the potential role that light scattering measurements have to play in future studies of cell death biology are presented. We first show that mitochondrial-PDT-induced morphology changes measured with light scattering map into the cell killing efficacy of the therapy. We next demonstrate that mitochondrial
Interactive directional subsurface scattering and transport of emergent light
DEFF Research Database (Denmark)
Dal Corso, Alessandro; Frisvad, Jeppe Revall; Mosegaard, Jesper;
2016-01-01
-based analytical models for subsurface scattering but also directional models. In addition, our method enables easy extraction of virtual point lights for transporting emergent light to the rest of the scene. Our method requires neither preprocessing nor texture parameterization of the translucent objects...... is the first to include interactive transport of emergent light from deformable translucent objects....
Light scattering from exoplanet oceans and atmospheres
Zugger, Michael E; Williams, Darren M; Kane, Timothy J; Philbrick, C Russell
2010-01-01
Orbital variation in polarized and unpolarized reflected starlight from exoplanets could eventually be used to detect liquid water on planet surfaces. Exoplanets with rough surfaces, or those dominated by atmospheric Rayleigh scattering, should reach peak brightness in full phase, orbital longitude (OL) = 180 degrees, whereas ocean-covered planets with transparent atmospheres should reach peak brightness in crescent phase near OL = 30 degrees. Application of Fresnel theory to a planet with no atmosphere covered by a calm ocean predicts a peak polarization fraction of 1 at OL = 74 degrees; however, our model shows that clouds, wind-driven waves, aerosols, absorption, and Rayleigh scattering in the atmosphere and within the water column, dilute the polarization fraction and shift the peak to other OLs. Observing at longer wavelengths reduces the obfuscation of the water polarization signature by Rayleigh scattering but does not mitigate the other effects. Planets with thick Rayleigh scattering atmospheres reach...
Light Scattering by Optically Soft Particles Theory and Applications
Sharma, Subodh K
2006-01-01
The present monograph deals with a particular class of approximation methods in the context of light scattering by small particles. This class of approximations has been termed as eikonal or soft particle approximations. The eikonal approximation was studied extensively in the potential scattering and then adopted in optical scattering problems. In this context, the eikonal and other soft particle approximations pertain to scatterers whose relative refractive index compared to surrounding medium is close to unity. The study of these approximations is very important because soft particles occur abundantly in nature. For example, the particles that occur in ocean optics, biomedical optics, atmospheric optics and in many industrial applications can be classified as soft particles. This book was written in recognition of the long-standing and current interest in the field of scattering approximations for soft particles. It should prove to be a useful addition for researchers in the field of light scattering.
Modelling of classical ghost images obtained using scattered light
Crosby, S.; Castelletto, S.; Aruldoss, C.; Scholten, R. E.; Roberts, A.
2007-08-01
The images obtained in ghost imaging with pseudo-thermal light sources are highly dependent on the spatial coherence properties of the incident light. Pseudo-thermal light is often created by reducing the coherence length of a coherent source by passing it through a turbid mixture of scattering spheres. We describe a model for simulating ghost images obtained with such partially coherent light, using a wave-transport model to calculate the influence of the scattering on initially coherent light. The model is able to predict important properties of the pseudo-thermal source, such as the coherence length and the amplitude of the residual unscattered component of the light which influence the resolution and visibility of the final ghost image. We show that the residual ballistic component introduces an additional background in the reconstructed image, and the spatial resolution obtainable depends on the size of the scattering spheres.
Optical scattering by a nonlinear medium, II: induced photonic crystal in a nonlinear slab of BBO
Godard, Pierre; Nicolet, Andre
2010-01-01
The purpose of this paper is to investigate the scattering by a nonlinear crystal whose depth is about the wavelength of the impinging field. More precisely, an infinite nonlinear slab is illuminated by an incident field which is the sum of three plane waves of the same frequency, but with different propagation vectors and amplitudes, in such a way that the resulting incident field is periodic. Moreover, the height of the slab is of the same order of the wavelength, and therefore the so-called slowly varying envelope approximation cannot be used. In our approach we take into account some retroactions of the scattered fields between them (for instance, we do not use the nondepletion of the pump beam). As a result, a system of coupled nonlinear partial differential equations has to be solved. To do this, the finite element method (FEM) associated with perfectly matched layers is well suited. Nevertheless, when using the FEM, the sources have to be located in the meshed area, which is of course impossible when d...
Jiang, Jinghua; McGraw, Greg; Ma, Ruiqing; Brown, Julie; Yang, Deng-Ke
2017-02-20
We developed a novel light enhancing film for an organic light emitting diode (OLED) based on polymer dispersed liquid crystal (PDLC). In the film, the liquid crystal droplets are unidirectionally aligned along the film normal direction and exhibit selective scattering. The film scatters light emitted only in directions with large incident angles but not light emitted in directions with small incident angles. When the light is scattered, it changes propagation direction and exits the OLED. The PDLC film reduces the total internal reflection and thus can significantly increase the light efficiency of the OLED.
Surface magnetism studied by polarized light emission after He+ scattering
Manske, J; Dirska, M; Lubinski, G; Schleberger, M; Narmann, A; Hoekstra, R
1997-01-01
Surface magnetism is studied by means of an ion beam of low energy (2-15 keV) scattered off the surface under grazing incidence conditions. During the scattering, a small fraction of the ions is neutralized into excited states which decay subsequently by light emission. The circular polarization of
Light scattering from polymer solutions and nanoparticle dispersions
Schärtl, Wolfgang; Janca, Josef
2007-01-01
Light scattering is a very powerful method to characterize the structure of polymers and nanoparticles in solution. Recent technical developments have strongly enhanced the possible applications of this technique, overcoming previous limitations like sample turbidity or insufficient experimental time scales. However, despite their importance, these new developments have not yet been presented in a comprehensive form. In addition, and maybe even more important to the broad audience, there lacks a simple-to-read textbook for students and non-experts interested in the basic principles and fundamental techniques of light scattering. As part of the Springer Laboratory series, this book tries not only to provide such a simple-to-read and illustrative textbook about the seemingly very complicated topic of light scattering from polymers and nanoparticles in dilute solution, but also intends to cover some of the newest technical developments in experimental light scattering.
Light scattering by neutrophils: model, simulation, and experiment.
Orlova, Darya Yu; Yurkin, Maxim A; Hoekstra, Alfons G; Maltsev, Valeri P
2008-01-01
We studied the elastic light-scattering properties of human blood neutrophils, both experimentally and theoretically. The experimental study was performed with a scanning flow cytometer measuring the light-scattering patterns (LSPs) of individual cells over an angular range of 5-60 deg. We determined the absolute differential light-scattering cross sections of neutrophils. We also proposed an optical model for a neutrophil as a sphere filled by small spheres and prolate spheroids that correspond to granules and segmented nucleus, respectively. This model was used in simulations of LSPs using the discrete dipole approximation and different compositions of internal organelles. A comparison of experimentally measured and simulated LSPs gives a good qualitative agreement in LSP shape and quantitative agreement in overall magnitude of the differential light-scattering cross section.
Light projectile scattering off the Color Glass Condensate
Fukushima, Kenji
2007-01-01
We systematically compute the expectation value of Wilson lines in the McLerran-Venugopalan model, which provides useful formulae for evaluation of the scattering aimplitude in the collision of a light projectile and a heavy target.
Analytic expression for in-field scattered light distribution
Peterson, Gary L.
2004-01-01
Light that is scattered from lenses and mirrors in an optical system produces a halo of stray light around bright objects within the field of view. The angular distribution of scattered light from any one component is usually described by the Harvey model. This paper presents analytic expressions for the scattered irradiance at a focal plane from optical components that scatter light in accordance with the Harvey model. It is found that the irradiance is independent of the location of an optical element within the system, provided the element is not located at or near an intermediate image plane. It is also found that the irradiance has little or no dependence on the size of the element.
Efficient light propagation for multiple anisotropic volume scattering
Energy Technology Data Exchange (ETDEWEB)
Max, N. [Lawrence Livermore National Lab., CA (United States)]|[California Univ., Davis, CA (United States)
1993-12-01
Realistic rendering of participating media like clouds requires multiple anisotropic light scattering. This paper presents a propagation approximation for light scattered into M direction bins, which reduces the ``ray effect`` problem in the traditional ``discrete ordinates`` method. For a volume of n{sup 3} elements, it takes O(M n{sup 3} log n + M{sup 2} n{sup 3}) time and O(M n{sup 3}) space.
Synthesis of aerogel tiles with high light scattering length
Danilyuk, A F; Okunev, A G; Onuchin, A P; Shaurman, S A
1999-01-01
The possibility of aerogel tiles production for RICH detectors is described. Monolithic blocks of silica aerogel were synthesized by two-step sol-gel processing of tetraethoxysilane Si(OEt) sub 4 followed by high temperature supercritical drying with organic solvent. The important characteristic of aerogel is the light scattering length. In the wide range of refraction indexes the light scattering length exceeds 4 cm at 400 nm.
Evaluation of advanced light scattering technology for microgravity experiments
Fredericks, W. J.; Rosenblum, W. M.
1990-01-01
The capabilities of modern light scattering equipment and the uses it might have in studying processes in microgravity are evaluated. Emphasis is on the resolution of polydisperse systems. This choice was made since a major use of light scattering was expected to be the study of crystal growth of macromolecules in low gravity environments. An evaluation of a modern photon correlation spectrometer and a Mie spectrometer is presented.
Visible light scatter as quantitative information source on milk constituents
DEFF Research Database (Denmark)
Melentieva, Anastasiya; Kucheryavskiy, Sergey; Bogomolov, Andrey
2012-01-01
-time monitoring of processes and products. Optical analysis is generally performed in near and middle infrared (NIR and MIR) regions and relies on the component absorbance and Beer’s Law. The light scatter effect is therefore considered as a disturbance to be avoided during the measurement or eliminated...... at the data analysis stage. The region of visible (Vis) light (400-800 nm) is economically attractive, because it offers a range of inexpensive light sources, optics and detectors. At present, however, it is commonly considered useless, because of the light scatter by fat globules (1-10 μm) and protein...
Application of light scattering to coatings a user's guide
Diebold, Michael P
2014-01-01
The book begins with the fundamentals of light scattering, first by individual particles, then by small groups of particles, and finally by the trillions of particles present in a real-life paint film. From there, Dr. Diebold focuses on application of these fundamentals to paint formulation. The scope includes both theory and practice with an emphasis on application (from both performance and cost standpoints). The book gives a clear understanding of light scattering principles and application of these principles to paint formulation (with a focus on TiO2 - the strongest scattering material a
Backward elastic light scattering of malaria infected red blood cells
Lee, Seungjun; Lu, Wei
2011-08-01
We investigated the backward light scattering pattern of healthy and malaria (Plasmodium falciparum) parasitized red blood cells. The spectrum could clearly distinguish between predominant ring stage infected blood cells and healthy blood cells. Further, we found that infected samples mixed with different stages of P. falciparum showed different signals, suggesting that even variance in parasite stages could also be detected by the spectrum. These results together with the backward scattering technique suggest the potential of non-invasive diagnosis of malaria through light scattering of blood cells near the surface of human body, such as using eyes or skin surface.
Scaling in light scattering by sharp conical metal tips
Pors, Anders; Bozhevolnyi, Sergey I
2016-01-01
Using the electrostatic approximation, we analyze electromagnetic fields scattered by sharp conical metal tips, which are illuminated with light polarized along the tip axis. We establish scaling relations for the scattered field amplitude and phase, whose validity is verified with numerical simulations. Analytic expressions for the wavelength, at which the scattered field near the tip changes its direction, and field decay near the tip extremity are obtained, relating these characteristics to the cone angle and metal permittivity. The results obtained have important implications to various tip-enhanced phenomena, ranging from Raman and scattering near-field imaging to photoemission spectroscopy and nano-optical trapping.
How to distinguish elastically scattered light from Stokes shifted light for solid-state lighting?
Meretska, M; Thyrrestrup, H; Mosk, A P; IJzerman, W L; Vos, W L
2015-01-01
We have studied the transport of light through phosphor diffuser plates that are used in commercial solid-state lighting modules (Fortimo). These polymer plates contain $\\mathrm{YAG:Ce}^{+3}$ phosphor particles that elastically scatter light and Stokes shifts it in the visible wavelength range (400-700 nm). We excite the phosphor with a narrowband light source, and measure spectra of the outgoing light. The Stokes shifted light is separated from the elastically scattered light in the measured spectra and using this technique we isolate the elastic transmission of the plates. This result allows us to extract the transport mean free path $l_{\\mathrm{tr}}$ over the full wavelength range by employing diffusion theory. Simultaneously, we determine the absorption mean free path $l_{\\mathrm{abs}}$ in the wavelength range 400 to 530 nm where $\\mathrm{YAG:Ce}^{+3}$ absorbs. The diffuse absorption $\\mu_{\\mathrm{a}} =\\frac{1}{l_{\\mathrm{abs}}}$ spectrum is qualitative similar to the absorption coefficient of $\\mathrm{YA...
Multiple scattering of polarized light: influence of absorption.
Hohmann, A; Voit, F; Schäfer, J; Kienle, A
2014-06-07
This work continues previous research about multiple scattering of polarized light propagation in turbid media, putting emphasis on the imaginary part of the scatterers' complex refractive index. The whole angle-dependent Müller matrix is evaluated by comparing results of a polarization sensitive radiative transfer solution to Maxwell theory. Turbid media of defined scatterer concentrations are modelled in three dimensions by sphere ensembles kept inside a cubic or spherical simulation volume. This study addresses the impact of absorption on polarization characteristics for selected media from low to high absorption. Besides that, effects caused by multiple and dependent scattering are shown for increasing volume concentration. In this context some unique properties associated with multiple scattering and absorption are pointed out. Further, scattering results in two dimensions are compared for examples of infinite parallel cylinders of high absorption and perpendicularly incident plane waves.
Light-induced scattering of light in NBS:Ce crystals
Voronov, V. V.; Dorosh, I. R.; Kuzminov, Iu. S.; Tkachenko, N. V.
1980-11-01
An experiment is described in which light-induced scattering of laser light was observed in Ce-doped (Sr/x/Ba/1-x/)/1-y/(Nb2O6)/y/ crystals with x = 0.61 and y = 0.4993. It is shown that the observed effect results from the holographic amplification of light scattered by crystal defects and that the observed asymmetry of the scattering is associated with the diffusion mechanism of hologram recording in crystals. A theoretical model of the scattering process is constructed for the diffusion recording mechanism.
Quantum noise memory effect of multiple scattered light
Lodahl, P
2005-01-01
We investigate frequency correlations in multiple scattered light that are present in the quantum fluctuations. The memory effect for quantum and classical noise is compared, and found to have markedly different frequency scaling, which was confirmed in a recent experiment. Furthermore, novel mesoscopic correlations are predicted that depend on the photon statistics of the incoming light.
Quantum noise frequency correlations of multiply scattered light
DEFF Research Database (Denmark)
Lodahl, Peter
2006-01-01
Frequency correlations in multiply scattered light that are present in quantum fluctuations are investigated. The speckle correlations for quantum and classical noise are compared and are found to depend markedly differently on optical frequency, which was confirmed in a recent experiment....... Furthermore, novel mesoscopic correlations are predicted that depend on the photon statistics of the incoming light....
Light scattering characteristicof TiO2 nanocrystalline porous films
Institute of Scientific and Technical Information of China (English)
无
2003-01-01
TiO2 nanocrystalline porous films consisting of binary particles mixture (mean diameters of 12 and 100 nm) are capable of increasing the light absorption due to the possession of large specific surface area and light scattering property. The simultaneous reduction of the film thickness leads to a decrease of the recombination loss during electron transport and an increase of the photocurrent efficiency.
Light scattering in optical CT scanning of Presage dosimeters
Energy Technology Data Exchange (ETDEWEB)
Xu, Y; Adamovics, J; Cheeseborough, J C; Chao, K S; Wuu, C S, E-mail: yx2010@columbia.ed
2010-11-01
The intensity of the scattered light from the Presage dosimeters was measured using a Thorlabs PM100D optical power meter (Thorlabs Inc, Newton, NJ) with an optical sensor of 1 mm diameter sensitive area. Five Presage dosimeters were made as cylinders of 15.2 cm, 10 cm, 4 cm diameters and irradiated with 6 MV photons using a Varian Clinac 2100EX. Each dosimeter was put into the scanning tank of an OCTOPUS' optical CT scanner (MGS Research Inc, Madison, CT) filled with a refractive index matching liquid. A laser diode was positioned at one side of the water tank to generate a stationary laser beam of 0.8 mm width. On the other side of the tank, an in-house manufactured positioning system was used to move the optical sensor in the direction perpendicular to the outgoing laser beam from the dosimeters at an increment of 1 mm. The amount of scattered photons was found to be more than 1% of the primary light signal within 2 mm from the laser beam but decreases sharply with increasing off-axis distance. The intensity of the scattered light increases with increasing light attenuations and/or absorptions in the dosimeters. The scattered light at the same off-axis distance was weaker for dosimeters of larger diameters and for larger detector-to-dosimeter distances. Methods for minimizing the effect of the light scattering in different types of optical CT scanners are discussed.
Comparative Study of Light Scattering from Hepatoma Cells and Hepatocytes
Lin, Xiaogang; Wang, Rongrong; Guo, Yongcai; Gao, Chao; Guo, Xiaoen
2012-11-01
Primary liver cancer is one of the highest mortality malignant tumors in the world. China is a high occurrence area of primary liver cancer. Diagnosis of liver cancer, especially early diagnosis, is essential for improving patients' survival. Light scattering and measuring method is an emerging technology developed in recent decades, which has attracted a large number of biomedical researchers due to its advantages, such as fast, simple, high accuracy, good repeatability, and non-destructive. The hypothesis of this project is that there may be some different light scattering information between hepatoma cells and hepatocyte. Combined with the advantages of the dynamic light scattering method and the biological cytology, an experimental scheme to measure the light scattering information of cells was formulated. Hepatoma cells and hepatic cells were irradiated by a semiconductor laser (532 nm). And the Brookhaven BI-200SM wide-angle light scattering device and temperature control apparatus were adopted. The light scattering information of hepatoma cells and hepatic cells in vitro within the 15°C to 30°C temperature range was processed by a BI-9000AT digital autocorrelator. The following points were found: (a) the scattering intensities of human hepatic cells and hepatoma cells are nearly not affected by the temperature factor, and the former is always greater than the latter and (b) the relaxation time of hepatoma cells is longer than that of hepatic cells, and both the relaxation time are shortened with increasing temperature from 15°C to 25°C. It can be concluded that hepatoma cells could absorb more incident light than hepatic cells. The reason may be that there exists more protein and nucleic acid in cancerous cells than normal cells. Furthermore, based on the length relaxation time, a conclusion can be inferred that the Brownian movement of cancer cells is greater.
Nonlinear light propagation in fs laser-written waveguide arrays
Directory of Open Access Journals (Sweden)
Szameit A.
2013-11-01
Full Text Available We report on recent achievements in the field of nonlinear light propagation in fs laser-written waveguide lattices. Particular emphasis is thereby given on discrete solitons in such systems.
Nonlinear quantum optics in the (ultra)strong light-matter coupling
Sánchez-Burillo, Eduardo; García-Ripoll, Juan José; Martín-Moreno, Luis; Zueco, David
2014-01-01
The propagation of $N$ photons in one dimensional waveguides coupled to $M$ qubits is discussed, both in the strong and ultrastrong qubit-waveguide coupling. Special emphasis is placed on the characterisation of the nonlinear response and its linear limit for the scattered photons as a function of $N$, $M$, qubit inter distance and light-matter coupling. The quantum evolution is numerically solved via the Matrix Product States technique. Both the time evolution for the field and qubits is com...
Ruan, Haowen; Yang, Changhuei
2015-01-01
Focusing light inside scattering media in a freely addressable fashion is challenging, as the wavefront of the scattered light is highly disordered. Recently developed ultrasound-guided wavefront shaping methods are addressing this challenge, albeit with relatively low modulation efficiency and resolution limitations. In this paper, we present a new technique, time-reversed ultrasound microbubble encoded (TRUME) optical focusing, which is able to focus light with improved efficiency and sub-ultrasound wavelength resolution. This method ultrasonically destructs microbubbles, and measures the wavefront change to compute and render a suitable time-reversed wavefront solution for focusing. We demonstrate that the TRUME technique can create an optical focus at the site of bubble destruction with a size of ~2 microns. Due to the nonlinear pressure-to-destruction response, the TRUME technique can break the addressable focus resolution barrier imposed by the ultrasound focus. We experimentally demonstrate a 2-fold ad...
Using light scattering to determine the stoichiometry of protein complexes.
Mogridge, Jeremy
2015-01-01
The stoichiometry of a protein complex can be calculated from an accurate measurement of the complex's molecular weight. Multiangle laser light scattering in combination with size exclusion chromatography and interferometric refractometry provides a powerful means for determining the molecular weights of proteins and protein complexes. In contrast to conventional size exclusion chromatography and analytical centrifugation, measurements do not rely on the use of molecular weight standards and are not affected by the shape of the proteins. The technique is based on the direct relationship between the amount of light scattered by a protein in solution, and the product of its concentration and molecular weight. A typical experimental configuration includes a size exclusion column to fractionate the sample, a light scattering detector to measure scattered light, and an interferometric refractometer to measure protein concentration. The determination of the molecular weight of an anthrax toxin complex will be used to illustrate how multiangle laser light scattering can be used to determine the stoichiometry of protein complexes.
Properties of nonreciprocal light propagation in a nonlinear optical isolator
Roy, Dibyendu
2016-01-01
Light propagation in a nonlinear optical medium is nonreciprocal for spatially asymmetric linear permittivity. We here examine physical mechanism and properties of such nonreciprocity (NR). For this, we calculate transmission of light through a two-level atom asymmetrically coupled to light inside open waveguides. We determine the critical intensity of incident light for maximum NR and a dependence of the corresponding NR on asymmetry in the coupling. Surprisingly, we find that it is mainly c...
Nonlinear optical absorption and stimulated Mie scattering in metallic nanoparticle suspensions
He, Guang S.; Law, Wing-Cheung; Baev, Alexander; Liu, Sha; Swihart, Mark T.; Prasad, Paras N.
2013-01-01
The nonlinear optical properties of four metallic (Au-, Au/Ag-, Ag-, and Pt-) nanoparticle suspensions in toluene have been studied in both femtosecond and nanosecond regimes. Nonlinear transmission measurements in the femtosecond laser regime revealed two-photon absorption (2PA) induced nonlinear attenuation, while in the nanosecond laser regime a stronger nonlinear attenuation is due to both 2PA and 2PA-induced excited-state absorption. In the nanosecond regime, at input pump laser intensities above a certain threshold value, a new type of stimulated (Mie) scattering has been observed. Being essentially different from all other well known molecular (Raman, Brillouin) stimulated scattering effects, the newly observed stimulated Mie scattering from the metallic nanoparticles exhibits the features of no frequency shift and low pump threshold requirement. A physical model of induced Bragg grating initiated by the backward Mie scattering from metallic nanoparticles is proposed to explain the gain mechanism of the observed stimulated scattering effect.
Light fields in complex media: Mesoscopic scattering meets wave control
Rotter, Stefan; Gigan, Sylvain
2017-01-01
The newly emerging field of wave front shaping in complex media has recently seen enormous progress. The driving force behind these advances has been the experimental accessibility of the information stored in the scattering matrix of a disordered medium, which can nowadays routinely be exploited to focus light as well as to image or to transmit information even across highly turbid scattering samples. An overview of these new techniques, their experimental implementations, and the underlying theoretical concepts following from mesoscopic scattering theory is provided. In particular, the intimate connections between quantum transport phenomena and the scattering of light fields in disordered media, which can both be described by the same theoretical concepts, are highlighted. Particular emphasis is put on how these topics relate to application-oriented research fields such as optical imaging, sensing, and communication.
LASER BIOLOGY AND MEDICINE: Light scattering study of rheumatoid arthritis
Beuthan, J.; Netz, U.; Minet, O.; Klose, Annerose D.; Hielscher, A. H.; Scheel, A.; Henniger, J.; Müller, G.
2002-11-01
The distribution of light scattered by finger joints is studied in the near-IR region. It is shown that variations in the optical parameters of the tissue (scattering coefficient μs, absorption coefficient μa, and anisotropy factor g) depend on the presence of the rheumatoid arthritis (RA). At the first stage, the distribution of scattered light was measured in diaphanoscopic experiments. The convolution of a Gaussian error function with the scattering phase function proved to be a good approximation of the data obtained. Then, a new method was developed for the reconstruction of distribution of optical parameters in the finger cross section. Model tests of the quality of this reconstruction method show good results.
Light dynamics in nonlinear trimers ans twisted multicore fibers
Castro-Castro, Claudia; Srinivasan, Gowri; Aceves, Alejandro B; Kevrekidis, Panayotis G
2016-01-01
Novel photonic structures such as multi-core fibers and graphene based arrays present unique opportunities to manipulate and control the propagation of light. Here we discuss nonlinear dynamics for structures with a few (2 to 6) elements for which linear and nonlinear properties can be tuned. Specifically we show how nonlinearity, coupling, and parity-time PT symmetric gain/loss relate to existence, stability and in general, dynamical properties of nonlinear optical modes. The main emphasis of our presentation will be on systems with few degrees of freedom, most notably couplers, trimers and generalizations thereof to systems with 6 nodes.
Inelastic light scattering in low dimensional semiconductors
Energy Technology Data Exchange (ETDEWEB)
Watt, M
1988-12-01
Raman scattering is a powerful technique with which to study the lattice vibrations of semiconductors. Investigations of the phonons of GalnAs-InP heterostructures have shown that although the phonons in GalnAs quantum wells resembled those of bulk GalnAs, they were screened by free carriers. Raman scattering and photoluminescence techniques were employed to estimate the plasma density at which plasmon-phonon coupling became significant. Triple crystal x-ray diffraction measurements complemented the Raman scattering data and provided information on the GalnAs alloy composition and state of strain. It was found that although nominally lattice-matched to the underlying InP, the epitaxially-grown layers were tetragonally distorted in the direction of growth. Assessment of sample damage produced by reactive-ion-etching (RIE) was undertaken as a prerequisite to the study of phonons in fabricated nanostructures. Structural damage to the crystal showed up as a relaxation of the crystalline selection rules allowing the observation of a symmetry-forbidden phonon. The intensity of this phonon correlated well with depth profiling of the damage. Optimised RIE conditions were found to produce negligible crystalline damage. The study of GaAs cylinders (with diameters of less than 100 nanometers) revealed an additional feature in the optical phonon region of their Raman spectra. This feature was identified as a surface phonon of the quantum cylinders. The experimentally-observed frequencies of the surface phonon peaks showed good agreement with calculated frequencies based on vibrations in small, geometrically-regular crystals. The main contribution of this work is the study of the surface phonons of the GaAs quantum cylinders. This is the first time that surface phonons have been observed in small fabricated samples: all previous work has involved specially-prepared crystalline powders or else comparatively large slab geometries. The conclusion that can be drawn from this work
Scattering of non-separable states of light
Reddy, Chithrabhanu P Salla Gangi; Singh, R P
2015-01-01
We experimentally show that the non-separability of polarization and orbital angular momentum present in a light beam remains preserved under scattering through a random medium like rotating ground glass. We verify this by measuring the degree of polarization and observing the intensity distribution of the beam when projected to different polarization states, before as well as after the scattering. We extend our study to the non-maximally non-separable states also.
Xue, Jin-Hua; Qian, Qiu-Mei; Wang, Yong-Sheng; Meng, Xia-Ling; Liu, Lu
2013-02-01
A novel method of resonance light scattering (RLS) was developed for the analysis of trace metallothioneins (MTs) in human urine. In a CH3COOH-CH3COONa buffer solution of pH 4.5, the formation of a complex between levofloxacin (LEV)-Pd and MTs led to enhance the RLS intensity of the system, and the enhanced RLS intensity at 468 nm was proportional to the concentration of MTs in the range of 0.059-22.4 μg mL-1. The linear regression equation was ΔI = 127.5 ρ (μg mL-1)-88.02 with a correlation coefficient of 0.9992, and the detection limit of 17.8 ng mL-1. The relative standard deviation and the average recovery were 3.8-5.4% (n = 11) and 92.15%, respectively. The proposed method is convenient, reliable and sensitive, and has been used successfully for the determination of trace MTs in human urine samples.
A Theory of Exoplanet Transits with Light Scattering
Robinson, Tyler D.
2017-02-01
Exoplanet transit spectroscopy enables the characterization of distant worlds, and will yield key results for NASA's James Webb Space Telescope. However, transit spectra models are often simplified, omitting potentially important processes like refraction and multiple scattering. While the former process has seen recent development, the effects of light multiple scattering on exoplanet transit spectra have received little attention. Here, we develop a detailed theory of exoplanet transit spectroscopy that extends to the full refracting and multiple scattering case. We explore the importance of scattering for planet-wide cloud layers, where the relevant parameters are the slant scattering optical depth, the scattering asymmetry parameter, and the angular size of the host star. The latter determines the size of the “target” for a photon that is back-mapped from an observer. We provide results that straightforwardly indicate the potential importance of multiple scattering for transit spectra. When the orbital distance is smaller than 10–20 times the stellar radius, multiple scattering effects for aerosols with asymmetry parameters larger than 0.8–0.9 can become significant. We provide examples of the impacts of cloud/haze multiple scattering on transit spectra of a hot Jupiter-like exoplanet. For cases with a forward and conservatively scattering cloud/haze, differences due to multiple scattering effects can exceed 200 ppm, but shrink to zero at wavelength ranges corresponding to strong gas absorption or when the slant optical depth of the cloud exceeds several tens. We conclude with a discussion of types of aerosols for which multiple scattering in transit spectra may be important.
Weak Turbulence in the Magnetosphere: Formation of Whistler Wave Cavity by Nonlinear Scattering
Crabtree, C; Ganguli, G; Mithaiwala, M; Galinsky, V; Shevchenko, V
2011-01-01
We consider the weak turbulence of whistler waves in the in low-\\beta\\ inner magnetosphere of the Earth. Whistler waves with frequencies, originating in the ionosphere, propagate radially outward and can trigger nonlinear induced scattering by thermal electrons provided the wave energy density is large enough. Nonlinear scattering can substantially change the direction of the wave vector of whistler waves and hence the direction of energy flux with only a small change in the frequency. A portion of whistler waves return to the ionosphere with a smaller perpendicular wave vector resulting in diminished linear damping and enhanced ability to pitch-angle scatter trapped electrons. In addition, a portion of the scattered wave packets can be reflected near the ionosphere back into the magnetosphere. Through multiple nonlinear scatterings and ionospheric reflections a long-lived wave cavity containing turbulent whistler waves can be formed with the appropriate properties to efficiently pitch-angle scatter trapped e...
Light scattering from macromolecular systems: Molecular crystals and polymers
Bernstein, E. R.
1981-11-01
The research objectives were to: (1) characterize phase transitions theoretically and experimentally in molecular crystal systems; (2) use the above understanding gained by light scattering studies and theoretical interpretation to apply to the more complex system of lyotropic liquid crystals; and (3) then apply knowledge gained on the model systems of increasing complexity to polymer liquid crystals and solid polymers as observed by laser light scattering techniques. Systems experimentally and theoretically discussed are: trioxane, triazine, benzil, and chloranil. Studies of lyotropic liquid crystals (sodium decyl sulfate, sodium sulfate, decanol, water) have progressed. The major findings are: a number of phase transitions occur between 20 and 60 C; these transitions evidence strong critical behavior and long correlation times for fluctuations; and liquid crystals can be studied by light scattering. Spectra of solid powders, ribbons, and liquid crystals of PBT and solid PBO were obtained.
Light losses from scattering in luminescent solar concentrator waveguides.
Breukers, Robert D; Smith, Gerald J; Stirrat, Hedley L; Swanson, Adam J; Smith, Trevor A; Ghiggino, Kenneth P; Raymond, Sebastiampillai G; Winch, Nicola M; Clarke, David J; Kay, Andrew J
2017-04-01
The reductions in the transmission of emission originating from a fluorophore dissolved in a polymer matrix due to light scattering were compared in two forms of planar waveguides used as luminescent solar concentrators: a thin film of poly(methylmethacrylate) (PMMA) spin-coated on a glass plate and a solid PMMA plate of the same dimensions. The losses attributable to light scattering encountered in the waveguide consisting of the thin film of polymer coated on a glass plate were not detectable within experimental uncertainty, whereas the losses in the solid polymer plate were significant. The losses in the solid plate are interpreted as arising from light-scattering centers comprising minute bubbles of vapor/gas, incomplete polymerization or water clusters that are introduced during or after the thermally induced polymerization process.
Light-by-light scattering in UPC at the LHC
Klusek-Gawenda, Mariola; Szczurek, Antoni
2016-01-01
We discuss diphoton semi(exclusive) production in ultraperipheral $PbPb$ collisions at energy of $\\sqrt{s_{NN}}=$ 5.5 TeV (LHC). The nuclear calculations are based on equivalent photon approximation in the impact parameter space. The cross sections for elementary $\\gamma \\gamma \\to \\gamma \\gamma$ subprocess are calculated including two different mechanisms: box diagrams with leptons and quarks in the loops and a VDM-Regge contribution with virtual intermediate hadronic excitations of the photons. We got relatively high cross sections in $PbPb$ collisions ($306$ nb). This opens a possibility to study the $\\gamma \\gamma \\to \\gamma \\gamma$ (quasi)elastic scattering at the LHC. We find that the cross section for elastic $\\gamma\\gamma$ scattering could be measured in the lead-lead collisions for the diphoton invariant mass $W_{\\gamma\\gamma} \\approx 15-20$ GeV.
Insulin association in neutral solutions studied by light scattering
DEFF Research Database (Denmark)
Hvidt, S.
1991-01-01
Molecular weights and weight distributions of sulfated, Zn-free, and 2Zn insulins have been measured at pH 7.3 as a function of concentration from 0.1 to 2 mg/ml by use of a combination of light scattering, refractometry, and size-exclusion chromatography. Results show that sulfated insulin is mo...... absence. An average hydrodynamic radius of 5.6 nm, close to the crystallographic size of the insulin hexamer, was determined from dynamic light scattering of 2Zn insulin solutions....
Nonspherical nanoparticles characterization by partially depolarized dynamic light scattering
Levin, Alexander D.; Shmytkova, Ekaterina A.
2015-06-01
The realization of improved depolarized dynamic light scattering method is presented. This technique supports measurement of non-spherical nanoparticals dimensions in liquids. The relations between translational and rotational diffusion coefficients and autocorrelation function of scattered light with polarized and depolarized components in various proportions are derived. Thus measurement of very weak cross-polarized component can be avoided. This improvement permits to reduce measurement time, to improve signal to noise ratio and results precision. The technique was applied for sizing of gold nanorods and multiwalled carbon nanotubes in liquids.
Dynamic light scattering with applications to chemistry, biology, and physics
Berne, Bruce J
2000-01-01
Lasers play an increasingly important role in a variety of detection techniques, making inelastic light scattering a tool of growing value in the investigation of dynamic and structural problems in chemistry, biology, and physics. Until the initial publication of this work, however, no monograph treated the principles behind current developments in the field.This volume presents a comprehensive introduction to the principles underlying laser light scattering, focusing on the time dependence of fluctuations in fluid systems; it also serves as an introduction to the theory of time correlation f
Effect of pyrophosphate on the light scatter in KDP crystal
Institute of Scientific and Technical Information of China (English)
无
2001-01-01
Pyrophosphate doped potassium dihydrogen phosphate (KDP) crystal was grown from aqueous solution by the temperature lowering method. Light scatter in KDP crystal was detected with the ultramicroscopic method. The light scatter in KDP crystal was aggravated when pyrophosphate was doped into the growth solution, which was distributed ununiformly in prism and pyramidal sectors of KDP crystal. Different effects of pyrophosphate on prism and pyramidal sectors of KDP crystal can explain this case. The transmission in this crystal was measured, showing that pyrophosphate affects the transmission evidently.
Second Harmonic Light Scattering from Macromolecules: Collagen.
Roth, Shmuel
In this work we present the theory and practice of optical second harmonic generation (SHG) as applied to rat-tail tendon collagen. Our work is the first quantitative application of SHG to biological systems. The angular dependence of SHG is found to display a sharp, intense, forward peak superimposed on a broad background. The sharp peak is shown to imply long-range polar order, while the broad background corresponds to that predicted for the random "up"/"down" array of collagen fibrils seen with the electron microscope. The dependence of fibril diameter distribution on age and state of hydration is measured. Our experiments also reveal information concerning the structure of the fibrils and their arrangement in the tendon. The degree of polar order, the coherence length of tendon for harmonic generation and the absolute magnitude of the nonlinear susceptibility of the collagen fibril are also determined. The biological significance of these findings and the many advantages of SHG for the structural study of biological macromolecules and tissues are discussed.
Compton scattering of twisted light: angular distribution and polarization of scattered photons
Stock, S; Fritzsche, S; Seipt, D
2015-01-01
Compton scattering of twisted photons is investigated within a non-relativistic framework using first-order perturbation theory. We formulate the problem in the density matrix theory, which enables one to gain new insights into scattering processes of twisted particles by exploiting the symmetries of the system. In particular, we analyze how the angular distribution and polarization of the scattered photons are affected by the parameters of the initial beam such as the opening angle and the projection of orbital angular momentum. We present analytical and numerical results for the angular distribution and the polarization of Compton scattered photons for initially twisted light and compare them with the standard case of plane-wave light.
An empirical correction for moderate multiple scattering in super-heterodyne light scattering
Botin, Denis; Mapa, Ludmila Marotta; Schweinfurth, Holger; Sieber, Bastian; Wittenberg, Christopher; Palberg, Thomas
2017-05-01
Frequency domain super-heterodyne laser light scattering is utilized in a low angle integral measurement configuration to determine flow and diffusion in charged sphere suspensions showing moderate to strong multiple scattering. We introduce an empirical correction to subtract the multiple scattering background and isolate the singly scattered light. We demonstrate the excellent feasibility of this simple approach for turbid suspensions of transmittance T ≥ 0.4. We study the particle concentration dependence of the electro-kinetic mobility in low salt aqueous suspension over an extended concentration regime and observe a maximum at intermediate concentrations. We further use our scheme for measurements of the self-diffusion coefficients in the fluid samples in the absence or presence of shear, as well as in polycrystalline samples during crystallization and coarsening. We discuss the scope and limits of our approach as well as possible future applications.
Inelastic light scattering in low dimensional semiconductors
Watt, M
1988-01-01
frequencies of the surface phonon peaks showed good agreement with calculated frequencies based on vibrations in small, geometrically-regular crystals. The main contribution of this work is the study of the surface phonons of the GaAs quantum cylinders. This is the first time that surface phonons have been observed in small fabricated samples: all previous work has involved specially-prepared crystalline powders or else comparatively large slab geometries. The conclusion that can be drawn from this work is that the cylinders are not only well-defined (as observed from the SEM micrographs) but they are also crystalline. The implication is that such structures can now be fabricated at a sufficiently high level to allow progress in prototype devices such as the quantum dot laser. Raman scattering is a powerful technique with which to study the lattice vibrations of semiconductors. Investigations of the phonons of GalnAs-InP heterostructures have shown that although the phonons in GalnAs quantum wells resembled t...
The Scattering Problem for a Noncommutative Nonlinear Schrödinger Equation
Directory of Open Access Journals (Sweden)
Bergfinnur Durhuus
2010-06-01
Full Text Available We investigate scattering properties of a Moyal deformed version of the nonlinear Schrödinger equation in an even number of space dimensions. With rather weak conditions on the degree of nonlinearity, the Cauchy problem for general initial data has a unique globally defined solution, and also has solitary wave solutions if the interaction potential is suitably chosen. We demonstrate how to set up a scattering framework for equations of this type, including appropriate decay estimates of the free time evolution and the construction of wave operators defined for small scattering data in the general case and for arbitrary scattering data in the rotationally symmetric case.
The linear and nonlinear optical effects of white light
Institute of Scientific and Technical Information of China (English)
QI XinYuan; LIU SiMin; GUO Ru; LU Yi; GAO YuanMei; LIU ZhaoHong; HUANG ChunFu; ZHANG XiaoHua; ZHU Nan; XU JingJun
2009-01-01
An overview of our research group's experimental and theoretical developments is provided on the linear and nonlinear optical effects of white light since 2003. Their work includes the experimental researches on the white light one-dimensional photovoltaic dark spatial solitons and the waveguides and directional couplers induced by them, the circular and elliptic white-light dark spatial solitons and the white-light photorefractive phase masks, two-dimensional white-light photonic lattices and the applications of the white-light dark spatial solitons in the digital image transmission field, the interaction between the two-dimensional white-light dark spatial solitons to enhance or to improve the correlateddegree of the white light through the interaction between the white-light beam and coherent dark spatial solitons, the interaction between the one-or two-dimensional white-light dark spatial solitons and the two-dimensional white-light photonic lattices, respectively. We also numerically simulate the interaction between two or more partially incoherent bright spatial solitons and the white bright spatial soliton pairs in the saturated logarithmic nonlinear medium. We have observed experimentally for the first time,the modulation instability of the coherent light and white light, respectively, in self-defocusing medium and so on.
The linear and nonlinear optical effects of white light
Institute of Scientific and Technical Information of China (English)
无
2009-01-01
An overview of our research group’s experimental and theoretical developments is provided on the linear and nonlinear optical effects of white light since 2003. Their work includes the experimental researches on the white light one-dimensional photovoltaic dark spatial solitons and the waveguides and directional couplers induced by them, the circular and elliptic white-light dark spatial solitons and the white-light photorefractive phase masks, two-dimensional white-light photonic lattices and the applications of the white-light dark spatial solitons in the digital image transmission field, the interaction between the two-dimensional white-light dark spatial solitons to enhance or to improve the correlated degree of the white light through the interaction between the white-light beam and coherent dark spatial solitons, the interaction between the one- or two-dimensional white-light dark spatial solitons and the two-dimensional white-light photonic lattices, respectively. We also numerically simulate the interaction between two or more partially incoherent bright spatial solitons and the white bright spatial soliton pairs in the saturated logarithmic nonlinear medium. We have observed experimentally for the first time, the modulation instability of the coherent light and white light, respectively, in self-defocusing medium and so on.
Light-by-light scattering sum rules in light of new data
Danilkin, Igor
2016-01-01
We evaluate the light-quark meson contributions to three exact light-by-light scattering sum rules in light of new data by the Belle Collaboration, which recently has extracted the transition form factors of the tensor meson $f_2(1270)$ as well as of the scalar meson $f_0(980)$. We confirm a previous finding that the $\\eta, \\eta^\\prime$ and helicity-2 $f_2(1270)$ contributions saturate one of these sum rules up to photon virtualities up to around 1 GeV$^2$. At larger virtualities, our sum rule analysis shows an important contribution of the $f_2(1565)$ meson and provides a first empirical extraction of its helicity-2 transition form factor. Two further sum rules allow us to predict the helicity-0 and helicity-1 transition form factors of the $f_2(1270)$ meson. Furthermore, our analysis also provides an update for the scalar and tensor meson hadronic light-by-light contributions to the muon's anomalous magnetic moment.
The impact of dust particle morphological details on light scattering
Kemppinen, Osku; Nousiainen, Timo; Lindqvist, Hannakaisa; Jeong, Gi Young
2016-04-01
We investigate the impact of dust particle surface roughness and internal structure on light scattering. Starting from digital representation of realistically shaped dust particles, we vary the particle morphology, and perform light scattering simulations to both the original and the modified particles. By mapping the changes in morphology to the changes in scattering, we will get information of how strongly and in which way a particular change affects scattering. All investigations have been done with complex, irregular particle shapes. For surface roughness studies we have kept the particle total volume virtually constant during the roughening process, and the roughness element size small enough to keep the overall shape relatively unchanged. For internal structure studies, the size and the external shape are kept constant. These safety measures help ensure that the effects seen are in fact due to the feature studied. The work is notable for model development, because some models can not include surface roughness, for example. In that case, the people who use such models have to adjust for the fact that the results are inaccurate, and by knowing how surface roughness typically changes the scattering results, the adjustment can be made. As a corollary, if it is shown that a particular feature does not change scattering results in any noticeable way, the model developers can confidently ignore or simplify it.
Development of bacterial colony phenotyping instrument using reflected scatter light
Doh, Iyll-Joon
Bacterial rapid detection using optical scattering technology (BARDOT) involves in differentiating elastic scattering pattern of bacterial colony. This elastic light scatter technology has shown promising label-free classification rate. However, there is limited success in certain circumstances where either a growth media or a colony has higher opacity. This situation is due to the physical principles of the current BARDOT which mainly relies on optical patterns generated by transmitted signals. Incoming light is obstructed and cannot be transmitted through the dense bacterial colonies, such as Lactobacillus, Yeast, mold and soil bacteria. Moreover, a blood agar, widely used in clinical field, is an example of an opaque media that does not allow light to be transmitted through. Therefore, in this research, a newly designed reflection type scatterometer is presented. The reflection type scatterometer measures the elastic scattering pattern generated by reflected signal. A theoretical model to study the optical pattern characteristic with respect to bacterial colony morphology is presented. Both theoretical and experiment results show good agreement that the size of backward scattering pattern has positive correlation to colony aspect ratio, a colony elevation to diameter ratio. Four pathogenic bacteria on blood agar, Escherichia coli K12, Listeria innocua, Salmonella Typhimurium, and Staphylococcus aureus, are tested and measured with proposed instrument. The measured patterns are analyzed with a classification software, and high classification rate can be achieved.
Properties of Differential Scattering Section Based on Multi-photon Nonlinear Compton Effect
Institute of Scientific and Technical Information of China (English)
无
2002-01-01
Properties of damping electrons in collision with photons based on multi-photon nonlinear Compton effect are investigated. The expressions of the differential scattering section are derived. Several useful conclusions are drawn.
Goertz, David E.; Frijlink, Martijn E.; de Jong, N.; van der Steen, A.F.W.
2006-01-01
An experimental lipid encapsulated contrast agent comprised substantially of micrometer to submicrometer diameter bubbles was evaluated for its capacity to produce nonlinear scattering in response to high transmit frequencies. Agent characterization experiments were conducted at transmit frequencies
Tunable scattering cancellation of light using anisotropic cylindrical cavities
Díaz-Aviñó, Carlos; Zapata-Rodríguez, Carlos J
2016-01-01
Engineered core-shell cylinders are good candidates for applications in invisibility and cloaking.In particular, hyperbolic nanotubes demonstrate tunable ultra-low scattering cross section in the visible spectral range. In this work we investigate the limits of validity of the condition for invisibility, which was shown to rely on reaching an epsilon near zero in one of the components of the effective permittivity tensor of the anisotropic metamaterial cavity. For incident light polarized perpendicularly to the scatterer axis, critical deviations are found in low-birefringent arrangements and also with high-index cores. We demonstrate that the ability of anisotropic metallodielectric nanocavities to dramatically reduce the scattered light is associated with a multiple Fano-resonance phenomenon. We extensively explore such resonant effect to identify tunable windows of invisibility.
Light scattering artefacts in a funnel phantom using optical CT
Energy Technology Data Exchange (ETDEWEB)
Bosi, Stephen G [Department of Radiation Oncology, Prince of Wales Hospital, Sydney (Australia); Brown, Saxby; Baldock, Clive [Institute of Medical Physics, School of Physics, University of Sydney Australia (Australia); Sarabipour, Sarvenaz [Department of Nuclear Medicine and Radiobiology, University of Sherbrooke (Canada); De Deene, Yves [Radiotherapy Department, Ghent University Hospital (Belgium)], E-mail: c.baldock@physics.usyd.edu.au
2009-05-01
A gelatin phantom containing a funnel-shaped region of high opacity (or optical density OD) was used to examine light-scattering induced artefacts in a cone-beam optical CT scanner used for gel dosimetry. To correctly simulate polymer gel dosimeters, the opacity was introduced by adding a colloidal scatterer to the gelatin. In line profiles of OD taken from 3-D reconstructions of the funnel, those profiles with a long pathlength through high OD regions exhibited a 'dishing' artefact, while those of short pathlength exhibited the opposite effect - 'doming'. These phenomena are accounted for by a model that includes the effect of stray, scattered light.
Hybrid graphene nematic liquid crystal light scattering device
Qasim, M. M.; Khan, A. A.; Kostanyan, A.; Kidambi, P. R.; Cabrero-Vilatela, A.; Braeuninger-Weimer, P.; Gardiner, D. J.; Hofmann, S.; Wilkinson, T. D.
2015-08-01
A hybrid graphene nematic liquid crystal (LC) light scattering device is presented. This device exploits the inherent poly-crystallinity of chemical vapour deposited (CVD) graphene films to induce directional anchoring and formation of LC multi-domains. This thereby enables efficient light scattering without the need for crossed polarisers or separate alignment layers/additives. The hybrid LC device exhibits switching thresholds at very low electric fields (crossed polarisers or separate alignment layers/additives. The hybrid LC device exhibits switching thresholds at very low electric fields (< 1 V μm-1) and repeatable, hysteresis free characteristics. This exploitation of LC alignment effects on CVD graphene films enables a new generation of highly efficient nematic LC scattering displays as well as many other possible applications. Electronic supplementary information (ESI) available. See DOI: 10.1039/c5nr04094a
Half a century of light scatter metrology and counting
Stover, John C.
2014-09-01
Back in the early days Bill Wolf once said something like: "The guy with the lowest scatter measurement is closest to the right answer." He was often right then - but not anymore. Everything has changed. Today measurements are limited by Rayleigh scatter from the air - not the instrument. We have both written and physical standards and everybody spells BRDF the same way. In the time it takes to give this talk, over 100,000 silicon wafers will be inspected around the world using a few thousand scatterometers - average price about one million dollars each. The way the world illuminates everything from homes to football fields is changing with the advent of high brightness LED's and these lighting systems are designed using a combination of scatter metrology and analysis techniques - many of which were started at The Optical Sciences Center. This paper reviews two major highlights in half a century of scatter metrology progress.
The Smoothness of Scattering Operators for Sinh-Gordon and Nonlinear Schrodinger Equations
Institute of Scientific and Technical Information of China (English)
Bao Xiang WANG
2002-01-01
We show that the scattering operator carries a band in Hs(Rn) × Hs-1(Rn) into Hs(Rn) ×Hs-1(Rn) for the sinh-Gordon equation and an analogous result also holds true for the nonlinearSchrodinger equation with an exponential nonlinearity, where s ≥ n/2 is arbitrary and n ≥ 2. Therefore,the scattering operators are infinitely smooth for the above two equations.
Asymmetrically pumped Bragg scattering with the effects of nonlinear phase modulation
DEFF Research Database (Denmark)
Andersen, Lasse Mejling; Friis, Søren Michael Mørk; Reddy, Dileep V.
2014-01-01
We derive exact solutions to asymmetrically pumped Bragg scattering with nonlinear phase-modulation (NPM) and show that this setup allows for the frequency conversion of many temporal modes, while reducing the effects due to NPM.......We derive exact solutions to asymmetrically pumped Bragg scattering with nonlinear phase-modulation (NPM) and show that this setup allows for the frequency conversion of many temporal modes, while reducing the effects due to NPM....
Optical Characterization of Optofluidic Waveguides Using Scattered Light Imaging.
Jenkins, Micah H; Phillips, Brian S; Zhao, Yue; Holmes, Matthew R; Schmidt, Holger; Hawkins, Aaron R
2011-08-01
The use of scattered light images is shown to be an attractive method for the characterization of optofluidic waveguides. The method is shown to be capable of measuring waveguide propagation losses and transmissions between solid and liquid-core structures. Measurement uncertainties are considered and characterized and were typically less than 15%.
HeNe-laser light scattering by human dental enamel
Zijp, [No Value; tenBosch, JJ; Groenhuis, RAJ
1995-01-01
Knowledge of the optical properties of tooth enamel and an understanding of the origin of these properties are necessary for the development of new optical methods for caries diagnosis and the measurement of tooth color. We measured the scattering intensity functions for HeNe-laser light of 80- to 1
Light scattering of PMMA latex particles in benzene: structural effects
Nieuwenhuis, E.A.; Vrij, A.
1979-01-01
Intra- and interparticle structural effects were studied in polymethylmethacrylate (PMMA) latex dispersions in a nonpolar solvent with the technique of light scattering. The required transparency of the dispersions was attained by a close matching of the refractive index of PMMA and solvent, for whi
Light scattering by photonic crystals with a dirac spectrum
Sepkhanov, Ruslan
2009-01-01
In this thesis we consider several effects of a Dirac spectrum in photonic crystals on the scattering and propagation of light. We calculate the effect of a Dirac point (a conical singularity in the band structure) on the transmission of radiation through a photonic crystal. We find that the transmi
Multiple scattering of polarized light in a turbid medium
Gorodnichev, E. E.; Kuzovlev, A. I.; Rogozkin, D. B.
2007-01-01
It is shown that multiple scattering of polarized light in a turbid medium can be represented as independent propagation of three basic modes: intensity and linearly and circularly polarized modes. Weak interaction between the basic modes can be described by perturbation theory and gives rise to "ov
Light scattering by photonic crystals with a dirac spectrum
Sepkhanov, Ruslan
2009-01-01
In this thesis we consider several effects of a Dirac spectrum in photonic crystals on the scattering and propagation of light. We calculate the effect of a Dirac point (a conical singularity in the band structure) on the transmission of radiation through a photonic crystal. We find that the
Quantum correlations induced by multiple scattering of quadrature squeezed light
DEFF Research Database (Denmark)
Lodahl, Peter
2006-01-01
Propagating quadrature squeezed light through a multiple scattering random medium is found to induce pronounced spatial quantum correlations that have no classical analogue. The correlations are revealed in the number of photons transported through the sample that can be measured from the intensity...
Using Light Scattering to Track, Characterize and Manipulate Colloids
van Oostrum, P.D.J.
2011-01-01
A new technique is developed to analyze in-line Digital Holographic Microscopy images, making it possible to characterize, and track colloidal particles in three dimensions at unprecedented accuracy. We took digital snapshots of the interference pattern between the light scattered by micrometer
Nonlinear optical signals and spectroscopy with quantum light
Dorfman, Konstantin E; Mukamel, Shaul
2016-01-01
Conventional nonlinear spectroscopy uses classical light to detect matter properties through the variation of its response with frequencies or time delays. Quantum light opens up new avenues for spectroscopy by utilizing parameters of the quantum state of light as novel control knobs and through the variation of photon statistics by coupling to matter. We present an intuitive diagrammatic approach for calculating ultrafast spectroscopy signals induced by quantum light, focusing on applications involving entangled photons with nonclassical bandwidth properties - known as "time-energy entanglement". Nonlinear optical signals induced by quantized light fields are expressed using time ordered multipoint correlation functions of superoperators. These are different from Glauber's g- functions for photon counting which use normally ordered products of ordinary operators. Entangled photon pairs are not subjected to the classical Fourier limitations on the joint temporal and spectral resolution. After a brief survey o...
Scattering optical elements: stand-alone optical elements exploiting multiple light scattering
Park, Jongchan; Park, Chunghyun; Lee, KyeoReh; Lee, Heon; Cho, Yong-Hoon; Park, YongKeun
2016-01-01
Optical design and fabrication techniques are crucial for making optical elements. From conventional lenses to diffractive optical elements, and to recent metasurfaces, various types of optical elements have been proposed to manipulate light where optical materials are fabricated into desired structures. Here, we propose a scattering optical element (SOE) which exploits multiple light scattering and wavefront shaping. Instead of fabricating optical materials, the SOE consists of a disordered medium and a photopolymer-based wavefront recorder, with shapes the wavefront of impinging light on demand. With the proposed stand-alone SOEs, we experimentally demonstrate control of various properties of light, including intensity, polarisation, spectral frequency and near field. Due to the tremendous freedom brought about by disordered media, the proposed approach will provide unexplored routes to manipulate arbitrary optical fields in stand-alone optical elements.
Energy Technology Data Exchange (ETDEWEB)
Zhou, Dong-Ying; Shi, Xiao-Bo; Gao, Chun-Hong; Cai, Shi-Duan; Jin, Yue; Liao, Liang-Sheng, E-mail: lsliao@suda.edu.cn
2014-09-30
Graphical abstract: - Highlights: • A combination of scattering layer and roughened substrate is used for light extraction from OLEDs. • The scattering layer is readily achieved by spin-coating the TiO{sub 2} sol. • The enhancement relying scattering depends on the size of TiO{sub 2} nano particles. • With the light extraction techniques the uniform emission is achieved. - Abstract: A combination of a scattering medium layer and a roughened substrate was proposed to enhance the light extraction efficiency of organic light-emitting diodes (OLEDs). Comparing with a reference OLED without any scattering layer, 65% improvement in the forward emission has been achieved with a scattering layer formed on an intentionally roughened external substrate surface of the OLED by spin-coating a sol–gel fabricated matrix containing well dispersed titania (TiO{sub 2}) particles. Such a combination method not only demonstrated efficient extraction of the light trapped in the glass substrate but also achieved homogenous emission from the OLED panel. The proposed technique, convenient and inexpensive, is believed to be suitable for the large area OLED production in lighting applications.
Kiselev, A D; Reshetnyak, V Yu; Sluckin, T J
2002-05-01
We extend the T-matrix approach to light scattering by spherical particles to some simple cases in which the scatterers are optically anisotropic. Specifically, we consider cases in which the spherical particles include radially and uniformly anisotropic layers. We find that in both cases the T-matrix theory can be formulated using a modified T-matrix ansatz with suitably defined modes. In a uniformly anisotropic medium we derive these modes by relating the wave packet representation and expansions of electromagnetic field over spherical harmonics. The resulting wave functions are deformed spherical harmonics that represent solutions of the Maxwell equations. We present preliminary results of numerical calculations of the scattering by spherical droplets. We concentrate on cases in which the scattering is due only to the local optical anisotropy within the scatterer. For radial anisotropy we find that nonmonotonic dependence of the scattering cross section on the degree of anisotropy can occur in a regime to which both the Rayleigh and semiclassical theories are inapplicable. For uniform anisotropy the cross section is strongly dependent on the angle between the incident light and the optical axis, and for larger droplets this dependence is nonmonotonic.
Disordered Cellulose-Based Nanostructures for Enhanced Light Scattering
2017-01-01
Cellulose is the most abundant biopolymer on Earth. Cellulose fibers, such as the one extracted form cotton or woodpulp, have been used by humankind for hundreds of years to make textiles and paper. Here we show how, by engineering light–matter interaction, we can optimize light scattering using exclusively cellulose nanocrystals. The produced material is sustainable, biocompatible, and when compared to ordinary microfiber-based paper, it shows enhanced scattering strength (×4), yielding a transport mean free path as low as 3.5 μm in the visible light range. The experimental results are in a good agreement with the theoretical predictions obtained with a diffusive model for light propagation. PMID:28191920
Functional Imaging of Tissue Morphology with Polarized Light Scattering Spectroscopy
Backman, Vadim
2001-03-01
We report a new imaging technique to study the morphology of living epithelial cells in vivo. The method is based on light scattering spectroscopy with polarized light (PLSS) and makes it possible to distinguish between single backscattering from epithelial cell nuclei and multiply scattered light. The spectrum of the single backscattering component is further analyzed to provide quantitative histological information about the epithelial cells such as the size distribution, refractive index, and chromatin content of the cell nuclei. The measurement of cell nuclear morphology is crucial for detection and diagnosis of cancerous and precancerous conditions in many human tissues. The method was successfully applied to image precancerous regions of several tissues. Clinical studies in five organs (esophagus, colon, bladder, oral cavity, and uterine cervix) showed the generality and efficacy of the technique.
Shape-dependent light scattering properties of subwavelength silicon nanoblocks.
Ee, Ho-Seok; Kang, Ju-Hyung; Brongersma, Mark L; Seo, Min-Kyo
2015-03-11
We explore the shape-dependent light scattering properties of silicon (Si) nanoblocks and their physical origin. These high-refractive-index nanostructures are easily fabricated using planar fabrication technologies and support strong, leaky-mode resonances that enable light manipulation beyond the optical diffraction limit. Dark-field microscopy and a numerical modal analysis show that the nanoblocks can be viewed as truncated Si waveguides, and the waveguide dispersion strongly controls the resonant properties. This explains why the lowest-order transverse magnetic (TM01) mode resonance can be widely tuned over the entire visible wavelength range depending on the nanoblock length, whereas the wavelength-scale TM11 mode resonance does not change greatly. For sufficiently short lengths, the TM01 and TM11 modes can be made to spectrally overlap, and a substantial scattering efficiency, which is defined as the ratio of the scattering cross section to the physical cross section of the nanoblock, of ∼9.95, approaching the theoretical lowest-order single-channel scattering limit, is achievable. Control over the subwavelength-scale leaky-mode resonance allows Si nanoblocks to generate vivid structural color, manipulate forward and backward scattering, and act as excellent photonic artificial atoms for metasurfaces.
Aerosol light scattering measurements as a function of relative humidity.
Day, D E; Malm, W C; Kreidenweis, S M
2000-05-01
The hygroscopic nature of atmospheric fine aerosol was investigated at a rural site in the Great Smoky Mountains National Park during July and August 1995. Passing the sample aerosol through an inlet, which housed an array of Perma Pure diffusion dryers, controlled the sample aerosol's relative humidity (RH). After conditioning the aerosol sample in the inlet, the light scattering coefficient and the aerosol size distribution were simultaneously measured. During this study, the conditioned aerosol's humidity ranged between 5% < RH < 95%. Aerosol response curves were produced using the ratio bspw/bspd; where bspw is the scattering coefficient measured at some RH greater than 20% and bspd is the scattering coefficient of the "dry" aerosol. For this work, any sample RH values below 15% were considered dry. Results of this investigation showed that the light scattering ratio increased continuously and smoothly over the entire range of relative humidity. The magnitude of the ratio at a particular RH value, however, varied considerably in time, particularly for RH values greater than approximately 60%. Curves of the scattering coefficient ratios as a function of RH were generated for each day and compared to the average 12-hour chemical composition of the aerosol. This comparison showed that for any particular RH value the ratio was highest during time periods of high sulfate concentrations and lowest during time periods of high soil or high organic carbon concentrations.
UV Nano Lights - Nonlinear Quantum Dot-Plasmon Coupling
2016-06-20
AFRL-AFOSR-JP-TR-2016-0072 UV Nano-Lights - Nonlinear Quantum Dot-Plasmon Coupling Eric Waclawik QUEENSLAND UNIVERSITY OF TECHNOLOGY Final Report 06...Final 3. DATES COVERED (From - To) 03 Feb 2014 to 02 Feb 2016 4. TITLE AND SUBTITLE UV Nano-Lights - Nonlinear Quantum Dot-Plasmon Coupling 5a...CONTRACT NUMBER 5b. GRANT NUMBER FA2386-14-1-4056 5c. PROGRAM ELEMENT NUMBER 61102F 6. AUTHOR(S) Eric Waclawik 5d. PROJECT NUMBER 5e. TASK NUMBER 5f
Light scattering by fractal dust aggregates: I. Angular dependence of scattering
Tazaki, Ryo; Okuzumi, Satoshi; Kataoka, Akimasa; Nomura, Hideko
2016-01-01
In protoplanetary disks, micron-sized dust grains coagulate to form highly porous dust aggregates. Because the optical properties of these aggregates are not completely understood, it is important to investigate how porous dust aggregates scatter light. In this study, the light scattering properties of porous dust aggregates were calculated using a rigorous method, the T-matrix method, and the results were then compared with those obtained using the Rayleigh-Gans-Debye (RGD) theory and Mie theory with the effective medium approximation (EMT). The RGD theory is applicable to moderately large aggregates made of nearly transparent monomers. This study considered two types of porous dust aggregates, ballistic cluster-cluster agglomerates (BCCAs) and ballistic particle-cluster agglomerates (BPCAs). First, the angular dependence of the scattered intensity was shown to reflect the hierarchical structure of dust aggregates; the large-scale structure of the aggregates is responsible for the intensity at small scatteri...
Evaluation of Influence of Multiple Scattering Effect in Light-Scattering-Based Applications
Institute of Scientific and Technical Information of China (English)
XU Sheng-Hua; SUN Zhi-Wei
2007-01-01
The extinction cross sections of a system containing two particles are calculated by the T-matrix method, and the results are compared with those of two single particles with single-scattering approximation. The necessity of the correction of the refractive indices of water and polystyrene for different incident wavelengths is particularly addressed in the calculation. By this means, the volume fractions allowed for certain accuracy requirements of single-scattering approximation in the light scattering experiment can be evaluated. The volume fractions calculated with corrected refractive indices are compared with those obtained with fixed refractive indices which have been rather commonly used, showing that fixed refractive indices may cause significant error in evaluating multiple scattering effect. The results also give a simple criterion for selecting the incident wavelength and particle size to avoid the 'blind zone' in the turbidity measurement, where the turbidity change is insensitive to aggregation of two particles.
Modulating light with light via giant nano-opto-mechanical nonlinearity of plasmonic metamaterial
Ou, Jun-Yu; Zhang, Jianfa; Zheludev, Nikolay I
2015-01-01
From the demonstration of saturable absorption by Vavilow and Levshin in 1926, and with invention of the laser, unavailability of strongly nonlinear materials was a key obstacle for developing optical signal processing, in particular in transparent telecommunication networks. Today, most advanced photonic switching materials exploit gain dynamics and near-band and excitonic effects in semiconductors, nonlinearities in organic media with weakly-localized electrons and nonlinearities enhanced by hybridization with metamaterials. Here we report on a new type of artificial nonlinearity that is nano-opto-mechanical in nature. It was observed in an artificial metamaterial array of plasmonic meta-molecules supported by a flexible nano-membrane. Here nonlinearity is underpinned by the reversible reconfiguration of its structure induced by light. In a film of only 100 nanometres thickness we demonstrated modulation of light with light using milliwatt power telecom diode lasers.
Using neural networks for dynamic light scattering time series processing
Chicea, Dan
2017-04-01
A basic experiment to record dynamic light scattering (DLS) time series was assembled using basic components. The DLS time series processing using the Lorentzian function fit was considered as reference. A Neural Network was designed and trained using simulated frequency spectra for spherical particles in the range 0–350 nm, assumed to be scattering centers, and the neural network design and training procedure are described in detail. The neural network output accuracy was tested both on simulated and on experimental time series. The match with the DLS results, considered as reference, was good serving as a proof of concept for using neural networks in fast DLS time series processing.
Geometrical optics approximation of light scattering by large air bubbles
Institute of Scientific and Technical Information of China (English)
Haitao Yu; Jianqi Shen; Yuehuan Wei
2008-01-01
For large spherical bubbles in water,geometrical optics approximation is considered a better method for calculating light scattering patterns.In this paper,the basic theory of geometrical optics approximation is clarified.The change of phase for bubbles is calculated when total reflection occurs,which is different from particles with relative refractive indices larger than 1.Verification of the method was achieved by assuming a spherical particle and comparing present results to Mie scattering and Debye calculation.Agreement with the Mie theory was excellent in all directions when the dimensionless size parameter is larger than 50.Limitations of the geometrical optics approximation are also discussed.
Institute of Scientific and Technical Information of China (English)
TONG Rui; WU Hui-Xia; QIU Xue-Qiong; QIAN Shi-Xiong; LIN Yang-Hui; CAI Rui-Fang
2006-01-01
@@ Three soluble polystyrene grafted multi-walled carbon nanotube (MWNT) samples are synthesized, and their optical performance and nonlinear scattering properties are investigated by z-scan method using nanosecond pulses of 532nm from a frequency-doubled Q-switched Nd:YLF laser. Analysis of the experimental results shows that other than nonlinear scattering, nonlinear absorption plays a major role in optical limiting performance of these stable and well-dispersed suspensions. These new synthesized materials which can be better dispersed in common organic solvents than MWNT itself can be considered as potential sources for further optical applications.
Free-form thin lens design with light scattering surfaces for practical LED down light illumination
Lin, Raychiy J.; Sun, Ching-Cherng
2016-05-01
The free-form optical quasilens surface technology was utilized to develop and design a solid transparent plastic optical lens for the LED down light with the narrow angular light distribution requirement in the LED lighting applications. In order to successfully complete the mission, the precise mid-field angular distribution model of the LED light source was established and built. And also the optical scattering surface property of the Harvey BSDF scattering model was designed, measured, and established. Then, the optical simulation for the entire optical system was performed to develop and design this solid transparent plastic optical lens system. Finally, the goals of 40 deg angular light distribution pattern defined at full width half maximum with glare reduced in the areas of interest and the optical performance of nearly 82% light energy transmission optics were achieved for the LED down light illumination.
Energy Technology Data Exchange (ETDEWEB)
Romero, MarIa de los Angeles Sandoval; Weder, Ricardo [Instituto de Investigaciones en Matematicas Aplicadas y en Sistemas, Universidad Nacional Autonoma de Mexico, Apartado Postal 20-726, Mexico DF 01000 (Mexico)
2006-09-15
We consider nonlinear Schroedinger equations with a potential, and non-local nonlinearities, that are models in mesoscopic physics, for example of a quantum capacitor, and that are also models of molecular structure. We study in detail the initial value problem for these equations, in particular, existence and uniqueness of local and global solutions, continuous dependence on the initial data and regularity. We allow for a large class of unbounded potentials. We have no restriction on the growth at infinity of the positive part of the potential. We also construct the scattering operator in the case of potentials that go to zero at infinity. Furthermore, we give a method for the unique reconstruction of the potential from the small amplitude limit of the scattering operator. In the case of the quantum capacitor, our method allows us to uniquely reconstruct all the physical parameters from the small amplitude limit of the scattering operator.
Optimization methods for characterization of single particles from light scattering patterns
Directory of Open Access Journals (Sweden)
M. A. Yurkin
2011-09-01
Full Text Available We address the inverse light-scattering problem for particles described by a several-parameters model, when experimental data are given as an angle-resolved lightscattering pattern (LSP. This problem is reformulated as an optimization (nonlinear regression problem, for which two solution methods are proposed. The first one is based on standard gradient optimization method, but with careful choice of the starting point. The second method is based on precalculated database of theoretical LSPs, from which the closest one to an experimental LSP is selected for characterization. We tested both methods for characterization of polystyrene microspheres using a scanning flow cytometer (SFC.
Light scattering from impurity enhanced liquid layers in polycrystalline ice
Thomson, E. S.; Wettlaufer, J. S.; Wilen, L. A.
2009-12-01
Impurity enhanced grain boundary premelting underlies a wide range of geophysical phenomena throughout the cryosphere. In particular, it is known that when water droplets freeze in the atmosphere they are highly polycrystalline and impurities are rejected into grain boundaries. The predicted character and sensitivity of grain boundaries to impurities close to the melting point precludes the use of standard techniques for imaging the interface. Unlike their larger more macroscopic relatives such as veins (3 grain intersections) and nodes (4 grain intersections), grain boundaries do not submit to optical microscopy. However, using an experimental light scattering method grain boundary changes can be measured as a function of thermodynamic variables. Accurate analysis of the light scattering data generated using this method requires a full theory of light propagation through the grain boundary layer straddled by ice crystals. Here we present a theory for light scattering from such a boundary, experimental data using NaCl as a dopant, and dicsuss atmospheric implications from the troposphere to the stratosphere.
Adaptive control of the propagation of ultrafast light through random and nonlinear media
Moores, Mark David
2001-12-01
Ultrafast light sources generate coherent pulses with durations of less than one picosecond, and represent the next generation of illuminators for medical imaging and optical communications applications. Such sources are already widely used experimentally. Correction of temporal widths or pulse envelopes after traversal of optically non-ideal materials is critical for the delivery of optimal ultrashort pulses. It is important to investigate the physical mechanisms that distort pulses and to develop and implement methods for minimizing these effects. In this work, we investigate methods for characterizing and manipulating pulse propagation dynamics in random (scattering) and nonlinear optical media. In particular, we use pulse shaping to manipulate the light field of ultrashort infrared pulses. Application of spectral phase by a liquid crystal spatial light modulator is used to control the temporal pulse shape. The applied phase is controlled by a genetic algorithm that adaptively responds to the feedback from previous phase profiles. Experiments are detailed that address related aspects of the character of ultrafast pulses-the short timescales and necessarily wide frequency bandwidths. Material dispersion is by definition frequency dependent. Passage through an inhomogeneous system of randomly situated boundaries (scatterers) causes additional distortion of ballistic pulses due to multiple reflections. The reflected rays accumulate phase shifts that depend on the separation of the reflecting boundaries and the photon frequency. Ultrafast bandwidths present a wide range of frequencies for dispersion and interaction with macroscopic dielectric structure. The shaper and adaptive learning algorithm are used to reduce these effects, lessening the impact of the scattering medium on propagating pulses. The timescale of ultrashort pulses results in peak intensities that interact with the electronic structure of optical materials to induce polarization that is no longer
de Aguiar, Hilton B; Brasselet, Sophie
2016-01-01
Despite the tremendous progresses in wavefront control through or inside complex scattering media, several limitations prevent reaching practical feasibility for nonlinear imaging in biological tissues. While the optimization of nonlinear signals might suffer from low signal to noise conditions and from possible artifacts at large penetration depths, it has nevertheless been largely used in the multiple scattering regime since it provides a guide star mechanism as well as an intrinsic compensation for spatiotemporal distortions. Here, we demonstrate the benefit of Transmission Matrix (TM) based approaches under broadband illumination conditions, to perform nonlinear imaging. Using ultrashort pulse illumination with spectral bandwidth comparable but still lower than the spectral width of the scattering medium, we show strong nonlinear enhancements of several orders of magnitude, through thicknesses of a few transport mean free paths, which corresponds to millimeters in biological tissues. Linear TM refocusing ...
Man, Weining; Fardad, Shima; Zhang, Ze; Prakash, Jai; Lau, Michael; Zhang, Peng; Heinrich, Matthias; Christodoulides, Demetrios N; Chen, Zhigang
2013-11-22
We demonstrate a new class of synthetic colloidal suspensions capable of exhibiting negative polarizabilities, and observe for the first time robust propagation and enhanced transmission of self-trapped light over long distances that would have been otherwise impossible in conventional suspensions with positive polarizabilities. Such light penetration through the strong scattering environment is attributed to the interplay between optical forces and self-activated transparency effects while no thermal effect is involved. By judiciously mixing colloidal particles of both negative and positive polarizabilities, we show that the resulting nonlinear response of these systems can be fine-tuned. Our experimental observations are in agreement with theoretical analysis based on a thermodynamic model that takes into account particle-particle interactions. These results may open up new opportunities in developing soft-matter systems with engineered optical nonlinearities.
Nonlinear metal-dielectric nanoantennas for light switching and routing
Noskov, R E; Kivshar, Yu S
2012-01-01
We introduce a novel hybrid metal-dielectric nanoantenna composed of dielectric (crystalline silicon) and metal (silver) nanoparticles. A high-permittivity dielectric nanoparticle allows to achieve effective light harvesting, and nonlinearity of a metal nanoparticle controls the radiation direction. We show that the radiation pattern of such a nanoantenna can be switched between the forward and backward directions by varying only the light intensity around the level of 11 MW/cm$^2$, with the characteristic switching time of 260 fs.
Nonlinear Propagation of Light in One Dimensional Periodic Structures
Goodman, Roy H.; Weinstein, Michael I.; Philip J Holmes
2000-01-01
We consider the nonlinear propagation of light in an optical fiber waveguide as modeled by the anharmonic Maxwell-Lorentz equations (AMLE). The waveguide is assumed to have an index of refraction which varies periodically along its length. The wavelength of light is selected to be in resonance with the periodic structure (Bragg resonance). The AMLE system considered incorporates the effects non-instantaneous response of the medium to the electromagnetic field (chromatic or material dispersion...
Light scattering from acoustic vibrational modes in confined structures
Bandhu, Rudra Shyam
The acoustic vibrational modes and their light scattering intensities in confined structures such as supported films, double layer free-standing membrane and sub-micron sized wires on a free-standing membrane have been studied using Brillouin Light Scattering (BLS). Standing wave type acoustic phonons were recently observed in supported thin films of silicon oxy-nitride. We build upon this finding to study the acoustic modes in thin zinc selenide (ZnSe) films on gallium arsenide (GaAs). The surprising behaviour of the Brillouin intensities of the standing wave modes in ZnSe are explained in terms of interference of the elasto-optic scattering amplitudes from the film and substrate. Numerical calculations of the scattering cross-section, which takes into account ripple and elasto-optic scattering mechanism, agrees well with the experimental data. Light scattering studies of standing wave type modes in free-standing polymethyl methacrylate (PMMA) layer on Si3N4 were carried out. In these bilayer structures PMMA is much softer than Si3N 4, a property that leads to confinement of low frequency modes associated with the PMMA layer to within its boundaries. In addition, the flexural and the dilatational modes from the Si3N4 layer are observed and are found to hybridize with the standing wave modes from the PMMA layer. Our study of phonon modes in PMMA wires supported on a free-standing Si3N4 membrane extends our work on free-standing double layer membranes. In recent years there is much interest in the study of phonon modes in nano-scale structures such as wires or dots. Although much theoretical work has been carried out in this direction, no experiments exist that explore the dispersion of the phonon modes in such structures. Brillouin Light scattering is ideally suited for studying phonons in such reduced dimensions and our work represents the first effort in this direction. The spectra reveal modes which are quantized both along the width, as well along the thickness
Angularly-resolved elastic light scattering of micro-particles
Aptowicz, Kevin B.
From microbiology to astrophysics, the scientific community has long embraced elastic light scattering from small particles as a diagnostic tool. Elastic light scattering has an extremely large scattering cross-section, allowing for single particle interrogation. This is critical in applications where trace amounts of suspect particles are to be detected in a diverse background of natural aerosols. By angularly-resolving the elastically scattered light, features can be detected in these patterns that are sensitive to a particle's morphology (shape, size, internal structure, and composition). An apparatus to collect LA TAOS (Large-Angle Two-dimensional Angular Optical Scattering) patterns from single particles in-situ and in real-time was designed and constructed. The setup utilizes a cross-beam trigger system to minimize the effects of the aberration coma stemming from the main collection optic, an ellipsoidal mirror. LA TAOS patterns of ambient aerosols were collected and analyzed. Approximately 15% of the ambient aerosol had a sphere-like shape. The refractive index of these spheres was estimated by curve-fitting to Lorenz-Mie theory. In addition, the island features prevalent in the LA TAOS pattern were analyzed. Metrics generated from these were used to get partial discrimination between clusters of Bacillus subtilis spores (a simulant for anthrax) and aerosol particles found in the ambient atmosphere. A novel experimental setup for collecting simultaneously LA TAOS patterns at two wavelengths in the mid-infrared was also implemented. With this setup, the relative strength of single-particle absorption could be discerned at the two illuminating wavelengths.
Supercontinuum Light Sources for Hyperspectral Subsurface Laser Scattering
DEFF Research Database (Denmark)
Nielsen, Otto Højager Attermann; Dahl, Anders Lindbjerg; Larsen, Rasmus;
2011-01-01
A materials structural and chemical composition influences its optical scattering properties. In this paper we investigate the use of subsurface laser scattering (SLS) for inferring structural and chemical information of food products. We have constructed a computer vision system based on a super......A materials structural and chemical composition influences its optical scattering properties. In this paper we investigate the use of subsurface laser scattering (SLS) for inferring structural and chemical information of food products. We have constructed a computer vision system based...... on a supercontinuum laser light source and an Acousto- Optic Tunable Filter (AOTF) to provide a collimated light source, which can be tuned to any wavelength in the range from 480 to 900 nm. We present the newly developed hyperspectral vision system together with a proof-of-principle study of its ability...... to discriminate between dairy products with either similar chemical or structural composition. The combined vision system is a new way for industrial food inspection allowing non-intrusive online process inspection of parameters that is hard with existing technology....
Quasielastic Light Scattering and Structure of Nanodroplets Mixed with Polycaprolactone
Directory of Open Access Journals (Sweden)
Soheil Sharifi
2014-01-01
Full Text Available The interaction of polycaprolactone (PCL with droplets of a microemulsion is studied with quasielastic light scattering and small angle X-ray scattering At constant droplet size we vary the PCL concentration and there is clear evidence for an increasing attractive interaction of the droplets from structural investigations with small-angle X-ray scattering (SAXS. The collective diffusion coefficient (Dc of the droplets is monitored with quasielastic light scattering (QELS. We mainly focus on the variation of the dynamic behavior as a function of the PCL concentration and length scale (M.W. = 5000 and 10000 in microemulsion. With increasing PCL concentration and length scale the dynamics of the system slow down. A hard sphere model with depletion potential can fit well the SAXS experiment of microemulsion mixed with PCL. The results show with increase of PCL on microemulsion the size of droplets is constant at 83Å but the size ratio of polymer to droplets is changing.
Light-scattering and dispersion behavior of multiwalled carbon nanotubes
Saltiel, Craig; Manickavasagam, Siva; Pinar Mengüc, M.; Andrews, Rodney
2005-08-01
Elliptically polarized light-scattering measurements were performed to investigate the dispersion behavior of multiwalled carbon nanotubes (MWNT). Xylene- and pyridine-derived MWNT powders were dispersed in water and ethanol in separate optic cells and allowed to sit undisturbed over a two-week time period after probe sonication. Continuous light-scattering measurements taken between scattering angles of 10-170 deg and repeated over several days showed that the nanotubes formed fractal-like networks. The pyridine-derived MWNTs showed greater dispersion variation over time, tending to aggregate and clump much faster than the xylene-derived tubes. The water suspensions appeared much more stable than the ethanol suspensions, which transformed into nonfractal morphology after a few hours. We relate the dispersion stability to size and fringe patterns on the outer surface of the nanotubes. Measured values of fractal dimension were distinctly lower than those in previous studies of single-walled carbon nanotubes. Profiles of both diagonal and off-diagonal scattering matrix elements are presented.
Application of a scattered-light radiometric power meter.
Caron, James N; DiComo, Gregory P; Ting, Antonio C; Fischer, Richard P
2011-04-01
The power measurement of high-power continuous-wave laser beams typically calls for the use of water-cooled thermopile power meters. Large thermopile meters have slow response times that can prove insufficient to conduct certain tests, such as determining the influence of atmospheric turbulence on transmitted beam power. To achieve faster response times, we calibrated a digital camera to measure the power level as the optical beam is projected onto a white surface. This scattered-light radiometric power meter saves the expense of purchasing a large area power meter and the required water cooling. In addition, the system can report the power distribution, changes in the position, and the spot size of the beam. This paper presents the theory of the scattered-light radiometric power meter and demonstrates its use during a field test at a 2.2 km optical range. © 2011 American Institute of Physics
Dynamic light scattering on bioconjugated laser generated gold nanoparticles.
Zimbone, Massimo; Baeri, Pietro; Calcagno, Lucia; Musumeci, Paolo; Contino, Annalinda; Barcellona, Maria Luisa; Bonaventura, Gabriele
2014-01-01
Gold nanoparticles (AuNPs) conjugated to DNA are widely used for biomedical targeting and sensing applications. DNA functionalization is easily reached on laser generated gold nanoparticles because of their unique surface chemistry, not reproducible by other methods. In this context, we present an extensive investigation concerning the attachment of DNA to the surface of laser generated nanoparticles using Dynamic Light Scattering and UV-Vis spectroscopy. The DNA conjugation is highlighted by the increase of the hydrodynamic radius and by the UV-Vis spectra behavior. Our investigation indicates that Dynamic Light Scattering is a suitable analytical tool to evidence, directly and qualitatively, the binding between a DNA molecule and a gold nanoparticle, therefore it is ideal to monitor changes in the conjugation process when experimental conditions are varied.
Dynamic light scattering on bioconjugated laser generated gold nanoparticles.
Directory of Open Access Journals (Sweden)
Massimo Zimbone
Full Text Available Gold nanoparticles (AuNPs conjugated to DNA are widely used for biomedical targeting and sensing applications. DNA functionalization is easily reached on laser generated gold nanoparticles because of their unique surface chemistry, not reproducible by other methods. In this context, we present an extensive investigation concerning the attachment of DNA to the surface of laser generated nanoparticles using Dynamic Light Scattering and UV-Vis spectroscopy. The DNA conjugation is highlighted by the increase of the hydrodynamic radius and by the UV-Vis spectra behavior. Our investigation indicates that Dynamic Light Scattering is a suitable analytical tool to evidence, directly and qualitatively, the binding between a DNA molecule and a gold nanoparticle, therefore it is ideal to monitor changes in the conjugation process when experimental conditions are varied.
Dust Evolution Can Produce Scattered Light Gaps in Protoplanetary Disks
Birnstiel, Tilman; Pinilla, Paola; Kama, Mihkel
2015-01-01
Recent imaging of protoplanetary disks with high resolution and contrast have revealed a striking variety of substructure. Of particular interest are cases where near-infrared scattered light images show evidence for low-intensity annular "gaps". The origins of such structures are still uncertain, but the interaction of the gas disk with planets is a common interpretation. We study the impact that the evolution of the solid material can have on the observable properties of disks in a simple scenario without any gravitational or hydrodynamical disturbances to the gas disk structure. Even with a smooth and continuous gas density profile, we find that the scattered light emission produced by small dust grains can exhibit ring-like depressions similar to those presented in recent observations. The physical mechanisms responsible for these features rely on the inefficient fragmentation of dust particles. The occurrence and position of the proposed "gap" features depend most strongly on the dust-to-gas ratio, the f...
Parhelic-like circle from light scattering in Plateau borders
Energy Technology Data Exchange (ETDEWEB)
Tufaile, A., E-mail: tufaile@usp.br; Tufaile, A.P.B.
2015-03-06
We are reporting a new simple optical element to generate halos. We have observed interesting patterns of light scattering in Plateau borders in foams. In analogy to the atmospheric phenomena known as parhelic circle, sun dogs, and sun pillars, we have named the features of the patterns observed as parlaseric circle, laser dogs, and laser pillars. The triangular symmetry of the Plateau borders is analogous to the hexagonal symmetry of ice crystals which produce these atmospheric phenomena. Working with one Plateau border at a time, we have observed wave optics phenomena that are not perceived in the atmospheric phenomena, such as diffraction and interference. - Highlights: • We obtained halo formation from light scattering in a Plateau border using an experiment. • We explained halo formation using geometrical theory of diffraction. • An optical element based on a Plateau border is proposed. • We compared some aspects of the parhelic circle with the parlaseric circle.
Extending Kubelka-Munk's Theory with Lateral Light Scattering
Mourad, Safer; Emmel, Patrick; Simon, Klaus; Hersch, Roger David
2001-01-01
Due to its simplicity, the theory of KUBELKA-MUNK [1] has found a wide acceptance for modeling the optical properties of light scattering materials. However, the concept is not explicitly adapted to predict halftone prints on paper. In this respect, a recent improvement was given by BERG. Our approach is an extension of BERG'S model in order to reduce the gap between the mathematical description of the paper's point spread function and the experimental results of simple reflectance measurements.
Dynamic Light Scattering Based Microelectrophoresis: Main Prospects and Limitations
Uskoković, Vuk
2012-01-01
Microelectrophoresis based on the dynamic light scattering (DLS) effect has been a major tool for assessing and controlling the conditions for stability of colloidal systems. However, both the DLS methods for characterization of the hydrodynamic size of dispersed submicron particles and the theory behind the electrokinetic phenomena are associated with fundamental and practical approximations that limit their sensitivity and information output. Some of these fundamental limitations, including...
Visible light scatter as quantitative information source on milk constituents
DEFF Research Database (Denmark)
Melentieva, Anastasiya; Kucheryavskiy, Sergey; Bogomolov, Andrey
2012-01-01
VISIBLE LIGHT SCATTER AS A QUANTITATIVE INFORMATION SOURCE ON MILK CONSTITUENTS A. Melenteva 1, S. Kucheryavski 2, A. Bogomolov 1,31Samara State Technical University, Molodogvardeyskaya Street 244, 443100 Samara, Russia. 2Aalborg University, campus Esbjerg, Niels Bohrs vej 8, 6700 Esbjerg, Denmar...... research area are presented and discussed. References: [1] A. Bogomolov, S. Dietrich, B. Boldrini, R.W. Kessler, Food Chemistry (2012), doi:10.1016/j.foodchem.2012.02.077....
Chahine algorithm to invert light scattering spectroscopy of epithelial dysplasia
Institute of Scientific and Technical Information of China (English)
无
2007-01-01
To perceive the epithelial dysplasia from the light scattering spectroscopy (LSS) is an inverse problem, which can be transformed into the inversion of the size distribution of epithelial-cell nuclei. Based on the simulation of single polarized LSS for epithelial-cell nuclei, Chahine algorithm is adopted to retrieve the size distribution. Numerical results show that Chahine algorithm has high inversion precision for both single-peaked and bimodal models, which implies the potential to increase diagnostic resolution of LSS.
Light scattering measurements supporting helical structures for chromatin in solution.
Campbell, A M; Cotter, R I; Pardon, J F
1978-05-01
Laser light scattering measurements have been made on a series of polynucleosomes containing from 50 to 150 nucleosomes. Radii of gyration have been determined as a function of polynucleosome length for different ionic strength solutions. The results suggest that at low ionic strength the chromatin adopts a loosely helical structure rather than a random coil. The helix becomes more regular on increasing the ionic strength, the dimension resembling those proposed by Finch and Klug for their solenoid model.
Ultraviolet refractometry using field-based light scattering spectroscopy
2009-01-01
Accurate refractive index measurement in the deep ultraviolet (UV) range is important for the separate quantification of biomolecules such as proteins and DNA in biology. This task is demanding and has not been fully exploited so far. Here we report a new method of measuring refractive index using field-based light scattering spectroscopy, which is applicable to any wavelength range and suitable for both solutions and homogenous objects with well-defined shape such as microspheres. The angula...
Computational analysis of light scattering from collagen fiber networks
Arifler, Dizem; Pavlova, Ina; Gillenwater, Ann; Richards-Kortum, Rebecca
2007-07-01
Neoplastic progression in epithelial tissues is accompanied by structural and morphological changes in the stromal collagen matrix. We used the Finite-Difference Time-Domain (FDTD) method, a popular computational technique for full-vector solution of complex problems in electromagnetics, to establish a relationship between structural properties of collagen fiber networks and light scattering, and to analyze how neoplastic changes alter stromal scattering properties. To create realistic collagen network models, we acquired optical sections from the stroma of fresh normal and neoplastic oral cavity biopsies using fluorescence confocal microscopy. These optical sections were then processed to construct three-dimensional collagen networks of different sizes as FDTD model input. Image analysis revealed that volume fraction of collagen fibers in the stroma decreases with neoplastic progression, and statistical texture features computed suggest that fibers tend to be more disconnected in neoplastic stroma. The FDTD modeling results showed that neoplastic fiber networks have smaller scattering cross-sections compared to normal networks of the same size, whereas high-angle scattering probabilities tend to be higher for neoplastic networks. Characterization of stromal scattering is expected to provide a basis to better interpret spectroscopic optical signals and to develop more reliable computational models to describe photon propagation in epithelial tissues.
High energy light scattering in the generalized eikonal approximation.
Chen, T W
1989-10-01
The generalized eikonal approximation method is applied to the study of light scattering by a dielectric medium. In this method, the propagation of light inside the medium is assumed to be rectilinear, as in the usual eikonal method, but with a parameterized propagator which is used to include the edge effect and ray optics behavior at the limit of very short wavelengths. The resulting formulas for the intensity and extinction efficiency factor are compared numerically and shown to agree excellently with the exact results for a homogeneous dielectric sphere.
Subdiffraction scattered light imaging of gold nanoparticles using structured illumination.
Chang, Bo-Jui; Lin, Shiuan Huei; Chou, Li-Jun; Chiang, Su-Yu
2011-12-15
A reflective light-scattering (RLS) microscope with structured illumination (SI) provides subdiffraction resolution and improves the image quality of gold nanoparticles in biological systems. The three-dimensional (3D)-structured pattern is rapidly and precisely controlled with a spatial light modulator and scrambled at the conjugate image plane to increase spatial incoherence. The reconstructed SI-RLS image of 100 nm gold nanoparticles reveals lateral and axial resolutions of approximately 117 and 428 nm. We present a high-resolution image of gold nanoparticles inside a HeLa cell, with improved contrast.
Metamaterials. Invisibility cloaking in a diffusive light scattering medium.
Schittny, Robert; Kadic, Muamer; Bückmann, Tiemo; Wegener, Martin
2014-07-25
In vacuum, air, and other surroundings that support ballistic light propagation according to Maxwell's equations, invisibility cloaks that are macroscopic, three-dimensional, broadband, passive, and that work for all directions and polarizations of light are not consistent with the laws of physics. We show that the situation is different for surroundings leading to multiple light scattering, according to Fick's diffusion equation. We have fabricated cylindrical and spherical invisibility cloaks made of thin shells of polydimethylsiloxane doped with melamine-resin microparticles. The shells surround a diffusively reflecting hollow core, in which arbitrary objects can be hidden. We find good cloaking performance in a water-based diffusive surrounding throughout the entire visible spectrum and for all illumination conditions and incident polarizations of light. Copyright © 2014, American Association for the Advancement of Science.
Propagation of coherent polarized light in turbid highly scattering medium.
Doronin, Alexander; Macdonald, Callum; Meglinski, Igor
2014-02-01
Within the framework of further development of unified Monte Carlo code for the needs of biomedical optics and biophotonics, we present an approach for modeling of coherent polarized light propagation in highly scattering turbid media, such as biological tissues. The temporal coherence of light, linear and circular polarization, interference, and the helicity flip of circularly polarized light due to reflection at the medium boundary and/or backscattering events are taken into account. To achieve higher accuracy in the results and to speed up the modeling, the implementation of the code utilizes parallel computing on NVIDIA graphics processing units using Compute Unified Device Architecture. The results of the simulation of coherent linearly and circularly polarized light are presented in comparison with the results of known theoretical studies and the results of alternative modelings.
Photovoltaic structures having a light scattering interface layer and methods of making the same
Energy Technology Data Exchange (ETDEWEB)
Liu, Xiangxin; Compaan, Alvin D.; Paudel, Naba Raj
2015-10-13
Photovoltaic (PV) cell structures having an integral light scattering interface layer configured to diffuse or scatter light prior to entering a semiconductor material and methods of making the same are described.
Determination of reversible protein equilibrium association coefficients using light scattering
Larkin, Michael
2009-03-01
The characterization in solution of reversible protein associations as well as associations between proteins and small molecules is essential in many areas of science. Understanding cellular function or developing and formulating pharmaceuticals or other biologically active materials often requires quantitation of such associations. Most pharmaceuticals have functionality due solely to association with molecules within the body, and the discovery and accurate characterization of these associations is a key element for pharmaceutical development. Unfortunately, most methods used to measure associations of proteins require either immobilizing the protein on a surface (e.g. surface plasmon resonance), which potentially alters the protein characteristics, or require considerable time and effort and large quantities of sample (e.g. analytical ultracentrifugation, isothermal titration calorimetry). Light scattering based measurements of reversible association coefficients require much less sample and may be performed much more rapidly than other free solution techniques. In this talk I describe how static and dynamic light scattering may each independently be used to measure equilibrium association coefficients between proteins in free solution, and may also be used to observe and quantitate the association of small molecules with them. I present background theory for both static and dynamic light scattering measurements of equilibrium associations, and examples of measurements made of both model systems and of systems with commercial relevance in the pharmaceutical industry.
Light scattering studies of solids and atomic vapors
Energy Technology Data Exchange (ETDEWEB)
Chiang, T.C.
1978-09-01
The general technique of light scattering and luminescence was used to study the properties of a number of material systems. First, multi-phonon resonant Raman scattering up to four phonons in GaSe and one- and two-phonon resonant Raman scattering in the mixed GaS/sub x/Se/sub 1-x/ crystals with x < or = 0.23 were investigated. Second, the observation of one-phonon resonant Raman scattering in HfS/sub 2/ is reported. The result is used to determine the position of the direct gap of HfS/sub 2/. Third, the first observation of the ..pi..-polarized one-magnon luminescence sideband of the /sup 4/T/sub lg/ (/sup 4/G) ..-->.. /sup 6/A/sub lg/(/sup 6/S) excitonic transition in antiferromagnetic MnF/sub 2/ is presented. An effective temperature of the crystal is deduced from the simultaneously observed anti-Stokes sideband emission. Multi-magnon (< or = 7) excitonic luminescence sidebands were also observed in MnF/sub 2/, KMnF/sub 2/, and RbMnF/sub 3/ using pulsed excitation and detection. A simple model based on two-ion local exchange is proposed to explain the results qualitatively. Fourth, the first observation of two-magnon resonant Raman scattering in MnF/sub 2/ around the magnon sidebands is reported. A simple theoretical description explains the experimental observations. Fifth, a detailed theory of exciton-exciton interaction in MnF/sub 2/ is developed to explain and to predict the experimental results on two-exciton absorption, high level excitation, and exciton--exciton scattering. Sixth, Brillouin scattering was used to obtain the five independent elastic constants of the layered compound GaSe. The results show clear elastic anisotropy of the crystal. Resonant Brillouin scattering near the absorption edge was also studied, but no resonant enhancement was found. Seventh, two-photon parametric scattering in sodium vapor was studied. Phase matching angles and scattering cross sections are calculated for a given set of experimental conditions.
Collision-induced light scattering in a thin xenon layer between graphite slabs - MD study.
Dawid, A; Górny, K; Wojcieszyk, D; Dendzik, Z; Gburski, Z
2014-08-14
The collision-induced light scattering many-body correlation functions and their spectra in thin xenon layer located between two parallel graphite slabs have been investigated by molecular dynamics computer simulations. The results have been obtained at three different distances (densities) between graphite slabs. Our simulations show the increased intensity of the interaction-induced light scattering spectra at low frequencies for xenon atoms in confined space, in comparison to the bulk xenon sample. Moreover, we show substantial dependence of the interaction-induced light scattering correlation functions of xenon on the distances between graphite slabs. The dynamics of xenon atoms in a confined space was also investigated by calculating the mean square displacement functions and related diffusion coefficients. The structural property of confined xenon layer was studied by calculating the density profile, perpendicular to the graphite slabs. Building of a fluid phase of xenon in the innermost part of the slot was observed. The nonlinear dependence of xenon diffusion coefficient on the separation distance between graphite slabs has been found.
Scattering in the ultrastrong regime: nonlinear optics with one photon
Sánchez-Burillo, Eduardo; Zueco, David; García-Ripoll, Juanjo; Martín-Moreno, Luis
2014-01-01
The scattering of a flying photon by a two-level system ultrastrongly coupled to a one-dimensional photonic waveguide is studied numerically. The photonic medium is modeled as an array of coupled cavities and the whole system is analyzed beyond the rotating wave approximation using Matrix Product States. It is found that the scattering is strongly influenced by the single- and multi-photon dressed bound states present in the system. In the ultrastrong coupling regime a new channel for inelast...
Light organization of small particles by multiple scattering
Hang, Zhi Hong
Optical manipulation is of broad interest in physics, chemistry, and biology. In the literature, most of the studies are focused on the optical trapping on a single object. In this thesis, we investigated the light-induced interaction of a collection of particles. The light-induced interaction between small particles was studied by a hierarchy of methods including the dipole theory, the multiple scattering and Maxwell stress tensor formalism, and the finite-difference-time-domain method. We showed that the multiple scattering between small particles could induce a binding mechanism to stabilize optically organized structures, but at the same time induced an intrinsic unbinding mechanism. The stability of optically organized structure was studied and a concept of "optical density" was introduced to gauge the destabilizing effect. We found that light-induced forces could bind dielectric spheres into extended structures through two mechanisms, each with its own length scale which could be adjusted by the configuration of the external light source. By manipulating the commensurability of the two length scales, these two mechanisms cooperated to bind a large number of spheres. When the two length scales became incommensurate for some particular incident angle, the competition between the two mechanisms led to modulated structures and other complex phenomena such as re-entrant stability. We searched for the possibility for stabilizing larger clusters. For this purpose, we found that circularly polarized light bound dielectric spheres into large-scale two-dimensional hexagonal lattice and multiple scattering also induced a rotation of optically bound structures. We searched for configurations that could induce optical trapping by field enhancement. Enhanced transmission on perforated metallic film system was studied. Surface modes bound on multi perforated perfect metal plate system were analytical solved and related to different high transmittance modes. Near
Lehtinen, K
2012-01-01
The optical surface brightness of dark nebulae is mainly due to scattering of integrated starlight by classical dust grains. It contains information on the impinging interstellar radiation field, cloud structure, and grain scattering properties. We have obtained spectra of the scattered light from 3500 to 9000 Angstrom in two globules, the Thumbprint Nebula and DC303.8-14.2. We use observations of the scattered light to study the impinging integrated starlight spectrum as well as the scattered H-alpha and other line emissions from all over the sky. We search also for the presence of other than scattered light in the two globules. We obtained long-slit spectra encompassing the whole globule plus adjacent sky in a one-slit setting, thus enabling efficient elimination of airglow and other foreground sky components. We calculated synthetic integrated starlight spectra for the solar neighbourhood using HIPPARCOS-based stellar distributions and the spectral library of Pickles. Spectra are presented separately for t...
Efficient Light Extraction from Organic Light-Emitting Diodes Using Plasmonic Scattering Layers
Energy Technology Data Exchange (ETDEWEB)
Rothberg, Lewis
2012-11-30
Our project addressed the DOE MYPP 2020 goal to improve light extraction from organic light-emitting diodes (OLEDs) to 75% (Core task 6.3). As noted in the 2010 MYPP, “the greatest opportunity for improvement is in the extraction of light from [OLED] panels”. There are many approaches to avoiding waveguiding limitations intrinsic to the planar OLED structure including use of textured substrates, microcavity designs and incorporating scattering layers into the device structure. We have chosen to pursue scattering layers since it addresses the largest source of loss which is waveguiding in the OLED itself. Scattering layers also have the potential to be relatively robust to color, polarization and angular distributions. We note that this can be combined with textured or microlens decorated substrates to achieve additional enhancement.
Michelson, Jennifer; Werner, Liliana; Ollerton, Andrew; Leishman, Lisa; Bodnar, Zachary
2012-08-01
To assess light scattering and light transmittance in intraocular lenses (IOLs) explanted because of optic opacification. John A. Moran Eye Center, University of Utah, Salt Lake City, Utah, USA. Experimental study. Poly(methyl methacrylate) (PMMA) IOLs with snowflake degeneration, hydrophilic acrylic IOLs with different calcification patterns, and 1 calcified silicone IOL explanted from an eye with asteroid hyalosis were studied with gross and light microscopy. Light scattering was measured with an EAS-1000 Scheimpflug camera. Light transmittance was measured with a Lambda 35 UV/Vis spectrophotometer (single-beam configuration with RSA-PE-20 integrating sphere). Analyses were performed at room temperature in the hydrated state and compared with controls. The study evaluated 8 PMMA IOLs, 22 hydrophilic acrylic IOLs, and 1 silicone IOL. Light scattering was as follows: 208 to 223 computer-compatible tapes (CCTs) for PMMA IOLs with snowflake degeneration (control = 9 CCTs); 90 to 227 CCTs for calcified hydrophilic acrylic IOLs (controls = 12 to 23 CCTs); 223 CCTs for the calcified silicone IOL (control = 5 CCTs). The mean light transmittance in the visible light spectrum was 81.08% to 97.10% for PMMA IOLs (control = 98.80%); 78.94% to 97.32% for hydrophilic acrylic IOLs (controls = 97.32% to 98.66%); 94.68% for the silicone IOL (control = 97.74%). Intraocular lens opacification led to very high levels of light scattering and a potential for decreased light transmittance, which play a role in the development of symptoms such as glare and halos, decreased contrast sensitivity, and eventually decreased visual acuity. No author has a financial or proprietary interest in any material or method mentioned. Copyright © 2012 ASCRS and ESCRS. Published by Elsevier Inc. All rights reserved.
LIGHT SOURCE: TW Laser system for Thomson scattering X-ray light source at Tsinghua University
Yan, Li-Xm; Du, Ying-Chao; Du, Qiang; Li, Ren-Kai; Hua, Jian-Fei; Huang, Wen-Hui; Tang, Chuan-Xiang
2009-06-01
A TW (Tera Watt) laser system based on Ti:sapphire mainly for the Tsinghua Thomson scattering X-ray light source (TTX) is being built. Both UV (ultraviolet) laser pulse for driving the photocathode radio-frequency (RF) gun and the IR (infrared) laser pulse as the electron-beam-scattered-light are provided by the system. Efforts have also been made in laser pulse shaping and laser beam transport to optimize the high-brightness electron beam production by the photocathode RF gun.
Cheng, Xing; Miao, Changxing; Zhao, Lifeng
2016-09-01
We consider the Cauchy problem for the nonlinear Schrödinger equation with combined nonlinearities, one of which is defocusing mass-critical and the other is focusing energy-critical or energy-subcritical. The threshold is given by means of variational argument. We establish the profile decomposition in H1 (Rd) and then utilize the concentration-compactness method to show the global wellposedness and scattering versus blowup in H1 (Rd) below the threshold for radial data when d ≤ 4.
Discovery of polarized light scattered by dust around Alpha Orionis
Mcmillan, R. S.; Tapia, S.
1978-01-01
Following the suggestion by Jura and Jacoby (1976), linearly polarized blue continuum starlight scattered by the dust shell around the M2 Iab star Alpha Orionis (Betelgeuse) has been discovered. The polarization has been traced in the NE, NW, SE, and SW directions and has positive (tangential) orientation. Some asymmetry of the optical depth in the shell exists 15 and 30 arcsec from the star. In the NE direction the polarization was measured as far as 90 arcsec (17,000 AU) from the star. The dependence of the average intensity of the scattered light from the nebula on angular distance from the star is more consistent with an inverse-square density law than with inverse 1.5 or inverse-cube laws. Assuming that the density is proportional to the inverse square of distance from the star, the scattering optical depth in blue light along a radius of 0.03 arcsec is no more than 0.15 + or - 0.05. Future observations of the wavelength dependence of polarization will allow a determination of grain size.
Inelastic light scattering spectroscopy of semiconductor nitride nanocolumns
Energy Technology Data Exchange (ETDEWEB)
Calleja, J.M.; Lazic, S.; Sanchez-Paramo, J. [Departamento de Fisica de Materiales, Universidad Autonoma de Madrid, 28049 Madrid (Spain); Agullo-Rueda, F. [Materials Science Institute of Madrid, CSIC, 28049 Madrid (Spain); Cerutti, L.; Ristic, J.; Fernandez-Garrido, S.; Sanchez-Garcia, M.A.; Grandal, J.; Calleja, E. [ISOM and Departamento de Ingenieria Electronica, ETSIT, Universidad Politecnica de Madrid, Ciudad Universitaria, 28040 Madrid (Spain); Trampert, A.; Jahn, U. [Paul-Drude-Institut fuer Festkoerperelektronik, Hausvogteiplatz 5-7, 10117 Berlin (Germany)
2007-08-15
A review of inelastic light scattering measurements on group III-nitride nanocolumns grown by molecular beam epitaxy is presented. The nanocolumns are hexagonal, high quality single crystals with diameters in the range of 20 to 100 nm, with no traces of extended defects. GaN nanocolumns grown on bare Si substrates with both (111) and (100) orientation display narrow phonon peaks, indicating the absence of strain inhomogeneities. This opens the possibility of efficient integration of the nanocolumns as optoelectronic devices with the complementary metal oxide semiconductor technology. Measurements of the E{sub 2} phonon frequency on AlGaN nanocolumns indicate a linear dependence of the Al concentration on the Al relative flux, up to 60%. The E{sub 2} peak width increases with Al content due to phonon damping by alloy scattering. Inelastic light scattering measurements in InN nanocolumns display a coupled LO phonon-plasmon mode together with uncoupled phonons. The coupled mode is not observed in a reference compact sample. The origin of the coupled mode is attributed to spontaneous accumulation of electrons at the lateral surfaces of the nanocolumns. The presence of free electrons in the nanocolumns is confirmed by infrared reflectance measurements. (copyright 2007 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)
Ultraviolet refractometry using field-based light scattering spectroscopy
Fu, Dan; Choi, Wonshik; Sung, Yongjin; Oh, Seungeun; Yaqoob, Zahid; Park, YongKeun; Dasari, Ramachandra R.; Feld, Michael S.
2010-01-01
Accurate refractive index measurement in the deep ultraviolet (UV) range is important for the separate quantification of biomolecules such as proteins and DNA in biology. This task is demanding and has not been fully exploited so far. Here we report a new method of measuring refractive index using field-based light scattering spectroscopy, which is applicable to any wavelength range and suitable for both solutions and homogenous objects with well-defined shape such as microspheres. The angular scattering distribution of single microspheres immersed in homogeneous media is measured over the wavelength range 260 to 315 nm using quantitative phase microscopy. By least square fitting the observed scattering distribution with Mie scattering theory, the refractive index of either the sphere or the immersion medium can be determined provided that one is known a priori. Using this method, we have measured the refractive index dispersion of SiO2 spheres and bovine serum albumin (BSA) solutions in the deep UV region. Specific refractive index increments of BSA are also extracted. Typical accuracy of the present refractive index technique is ≤0.003. The precision of refractive index measurements is ≤0.002 and that of specific refractive index increment determination is ≤0.01 mL/g. PMID:20372622
Ulku, Huseyin Arda
2015-02-01
An explicit marching on-in-time (MOT) based time domain electric field volume integral equation (TDVIE) solver for characterizing electromagnetic wave interactions on scatterers with nonlinear material properties is proposed. Discretization of the unknown electric field intensity and flux density is carried out by half and full Schaubert-Wilton-Glisson basis functions, respectively. Coupled system of spatially discretized TDVIE and the nonlinear constitutive relation between the field intensity and the flux density is integrated in time to compute the samples of the unknowns. An explicit PE(CE)m scheme is used for this purpose. Explicitness allows for \\'easy\\' incorporation of the nonlinearity as a function only to be evaluated on the right hand side of the coupled system of equations. A numerical example that demonstrates the applicability of the proposed MOT scheme to analyzing electromagnetic interactions on Kerr-nonlinear scatterers is presented. © 2015 IEEE.
Fractal analysis of the Rayleigh Photoinduced Light Scattering Pattern from LiNbO3:Zn Crystals
Sidorov, N. V.; Manukovskaya, D. V.; Palatnikov, M. N.
2017-03-01
Fractal analysis was used to study Rayleigh photoinduced light scattering (PILS) patterns in a series of LiNbO3:Zn single crystals (0.018-0.88 mass%) that were grown from the congruent melt and were promising as nonlinear optical materials with low photorefraction and coercive-field values. Results from fractal analysis and Raman light-scattering spectroscopy were compared. Extremes found on the time dependence of the fractal dimension of various layers of the PILS pattern speckle structure indicated that the concentration of laser-induced defects in the photorefractive crystal changed. The rate of change of the concentration of laser-induced defects depended non-linearly on the crystal Zn concentration. The form of congruent Zn-doped LiNbO3 crystals with the most ordered structure was identified.
The muon g-2: Dyson-Schwinger status on hadronic light-by-light scattering
Energy Technology Data Exchange (ETDEWEB)
Eichmann, Gernot; Fischer, Christian S.; Heupel, Walter; Williams, Richard [Institut für Theoretische Physik, Justus-Liebig–Universität Giessen, 35392 Giessen (Germany)
2016-01-22
We give a status report on the hadronic light-by-light scattering contribution to the muon’s anomalous magnetic moment from the Dyson-Schwinger approach. We discuss novel, model-independent properties of the light-by-light amplitude: we give its covariant decomposition in view of electromagnetic gauge invariance and Bose symmetry, and we identify the relevant kinematic regions that are probed under the integral. The decomposition of the amplitude at the quark level and the importance of its various diagrams are discussed and related to model approaches.
Stray-light suppression with high-collection efficiency in laser light-scattering experiments
Deilamian, K.; Gillaspy, J. D.; Kelleher, D. E.
1992-01-01
An optical system is described for collecting a large fraction of fluorescent light emitted isotropically from a cylindrical interaction region. While maintaining an overall detection efficiency of 9 percent, the system rejects, by more than 12 orders of magnitude, incident laser light along a single axis that intersects the interaction region. Such a system is useful for a wide variety of light-scattering experiments in which high-collection efficiency is desirable, but in which light from an incident laser beam must be rejected without resorting to spectral filters.
Neutron and light scattering studies of polymers adsorbed on laponite
Nelson, A R J
2002-01-01
The adsorption of poly(ethylene oxide) (PEO) and various poly(ethylene oxide)-poly(propylene oxide)-poly(ethylene oxide) (Pluronic) copolymers onto the synthetic clay Laponite, was investigated using Small Angle Neutron Scattering (SANS) and Dynamic Light Scattering (DLS). The Laponite particles are anisotropic, with a relatively high aspect ratio; but are the same order of magnitude in size as the polymer radius of gyration. Consequently, the particles present a radically different adsorption geometry compared to a locally planar interface, that is assumed by the majority of adsorption studies. The PEO homo-polymer formed thin layers, with the layer thickness being much smaller on the face than on the edge of the particle. Furthermore, the face thickness remained constant with increasing molecular weight, unlike the edge thickness, which grew with a small power law dependence on the molecular weight. Although the hydrodynamic thicknesses (DLS) were larger than those observed with SANS, the layer thicknesses ...
Light dark matter scattering in outer neutron star crusts
Cermeño, Marina; Silk, Joseph
2016-01-01
We calculate for the first time the phonon excitation rate in the outer crust of a neutron star due to scattering from light dark matter (LDM) particles gravitationally boosted into the star. We consider dark matter particles in the sub-GeV mass range scattering off a periodic array of nuclei through an effective scalar-vector interaction with nucleons. We find that LDM effects cause a modification of the net number of phonons in the lattice as compared to the standard thermal result. In addition, we estimate the contribution of LDM to the ion-ion thermal conductivity in the outer crust and find that it can be significantly enhanced at large densities. Our results imply that for magnetized neutron stars the LDM-enhanced global conductivity in the outer crust will tend to reduce the anisotropic heat conduction between perpendicular and parallel directions to the magnetic field.
Light dark matter scattering in outer neutron star crusts
Cermeño, Marina; Pérez-García, M. Ángeles; Silk, Joseph
2016-09-01
We calculate for the first time the phonon excitation rate in the outer crust of a neutron star due to scattering from light dark matter (LDM) particles gravitationally boosted into the star. We consider dark matter particles in the sub-GeV mass range scattering off a periodic array of nuclei through an effective scalar-vector interaction with nucleons. We find that LDM effects cause a modification of the net number of phonons in the lattice as compared to the standard thermal result. In addition, we estimate the contribution of LDM to the ion-ion thermal conductivity in the outer crust and find that it can be significantly enhanced at large densities. Our results imply that for magnetized neutron stars the LDM-enhanced global conductivity in the outer crust will tend to reduce the anisotropic heat conduction between perpendicular and parallel directions to the magnetic field.
Lee, Keunsoo; Shin, Jin-Wook; Park, Jun-Hwan; Lee, Jonghee; Joo, Chul Woong; Lee, Jeong-Ik; Cho, Doo-Hee; Lim, Jong Tae; Oh, Min-Cheol; Ju, Byeong-Kwon; Moon, Jaehyun
2016-07-13
We propose and fabricate a random light scattering layer for light extraction in organic light-emitting diodes (OLEDs) with silver nanodots, which were obtained by melting silver nanowires. The OLED with the light scattering layer as an internal light extraction structure was enhanced by 49.1% for the integrated external quantum efficiency (EQE). When a wrinkle structure is simultaneously used for an external light extraction structure, the total enhancement of the integrated EQE was 65.3%. The EQE is maximized to 65.3% at a current level of 2.0 mA/cm(2). By applying an internal light scattering layer and wrinkle structure to an OLED, the variance in the emission spectra was negligible over a broad viewing angle. Power mode analyses with finite difference time domain (FDTD) simulations revealed that the use of a scattering layer effectively reduced the waveguiding mode while introducing non-negligible absorption. Our method offers an effective yet simple approach to achieve both efficiency enhancement and spectral stability for a wide range of OLED applications.
Photonics linear and nonlinear interactions of laser light and matter
Menzel, R
2007-01-01
This book covers the fundamental properties and the description of single photons and light beams, experimentally and theoretically. It explains the essentials of linear interactions and most nonlinear interactions between light and matter in both the transparent and absorbing cases. It also provides a basic understanding of modern quantum optics and lasers, as well as the principles of nonlinear optical spectroscopy. It is self-consistent and enriched by a large number of calculated illustrations, examples, and descriptive tables. Graduate students in physics and electrical engineering, as well as other sciences, will find this book a thorough introduction to the field, while for lecturers and scientists it is a rich source of useful information and a ready-to-hand reference. The new edition has been thoroughly expanded and revised in all sections
Mandel'shtam-Brillouin scattering of laser light as a remote sensing tool.
Daniels, A.
1972-01-01
The mathematical relations regarding the intensity of scattered light are derived. The nature of density inhomogeneities in air is discussed together with scattering due to moving isothermal pressure fluctuations, the spectral distribution of scattering from static isobaric density fluctuations, and applications of Mandel'shtam-Brillouin (M-B) scattering to atmospheric sensing. It is concluded that M-B scattering of laser light from the atmosphere has an outstanding potential for remote atmospheric sensing.
Population of collective modes in light scattering by many atoms
Guerin, William; Kaiser, Robin
2017-05-01
The interaction of light with an atomic sample containing a large number of particles gives rise to many collective (or cooperative) effects, such as multiple scattering, superradiance, and subradiance, even if the atomic density is low and the incident optical intensity weak (linear optics regime). Tracing over the degrees of freedom of the light field, the system can be well described by an effective atomic Hamiltonian, which contains the light-mediated dipole-dipole interaction between atoms. This long-range interaction is at the origin of the various collective effects, or of collective excitation modes of the system. Even though an analysis of the eigenvalues and eigenfunctions of these collective modes does allow distinguishing superradiant modes, for instance, from other collective modes, this is not sufficient to understand the dynamics of a driven system, as not all collective modes are significantly populated. Here, we study how the excitation parameters, i.e., the driving field, determines the population of the collective modes. We investigate in particular the role of the laser detuning from the atomic transition, and demonstrate a simple relation between the detuning and the steady-state population of the modes. This relation allows understanding several properties of cooperative scattering, such as why superradiance and subradiance become independent of the detuning at large enough detuning without vanishing, and why superradiance, but not subradiance, is suppressed near resonance. We also show that the spatial properties of the collective modes allow distinguishing diffusive modes, responsible for radiation trapping, from subradiant modes.
Dynamic light scattering in veterinary medicine: refinement of diagnostic criteria
Dubin, Stephen; Zietz, Stanley; Gabriel, Karl L.; Gabriel, David; DellaVecchia, Michael A.; Ansari, Rafat R.
2001-05-01
In dynamic light scattering (DLS), the structure or material of interest, suspended in a fluid, is illuminated by a beam of laser light and the scattered light is interpreted in terms of diffusion coefficient, particle size or its distribution. DLS has shown clear promise as a non-invasive, objective and precise diagnostic modality for investigation of lens opacity (cataract) and other medical and toxicological problems. The clinical potential of LDS has been demonstrated in several species both in vivo and in vitro. In many clinical cases, discernment between normal and diseased patients is possible by simple inspection of the particle size distribution. However a more rigorous and sensitive classification scheme is needed, particularly for evaluation of therapy and estimation of tissue injury. The data supplied by DLS investigation is inherently multivariate and its most efficient interpretation requires a multivariate approach which includes the variability among specimens as well as any correlation among the variables (e.g. across the particle size distribution). We present a brief review of DLS methodology, illustrative data and our efforts toward a diagnostic classification scheme. In particular we will describe application of the Mahalanobis distance and related statistical methods to DLS data.
Enhanced Light Scattering of Secondary Organic Aerosols by Multiphase Reactions.
Li, Kun; Li, Junling; Liggio, John; Wang, Weigang; Ge, Maofa; Liu, Qifan; Guo, Yucong; Tong, Shengrui; Li, Jiangjun; Peng, Chao; Jing, Bo; Wang, Dong; Fu, Pingqing
2017-02-07
Secondary organic aerosol (SOA) plays a pivotal role in visibility and radiative forcing, both of which are intrinsically linked to the refractive index (RI). While previous studies have focused on the RI of SOA from traditional formation processes, the effect of multiphase reactions on the RI has not been considered. Here, we investigate the effects of multiphase processes on the RI and light-extinction of m-xylene-derived SOA, a common type of anthropogenic SOA. We find that multiphase reactions in the presence of liquid water lead to the formation of oligomers from intermediate products such as glyoxal and methylglyoxal, resulting in a large enhancement in the RI and light-scattering of this SOA. These reactions will result in increases in light-scattering efficiency and direct radiative forcing of approximately 20%-90%. These findings improve our understanding of SOA optical properties and have significant implications for evaluating the impacts of SOA on the rapid formation of regional haze, global radiative balance, and climate change.
Light-by-light scattering in the Lamb shift and the bound electron g factor
Czarnecki, Andrzej; Szafron, Robert
2016-12-01
We compute an O ( α2(Zα ) 6) contribution to the hydrogen-atom Lamb shift arising from light-by-light scattering. Analogous diagrams, with one atomic electric field insertion replaced by an external magnetic field, contribute to the gyromagnetic factor of the bound electron at O ( α2(Zα ) 4) . We also calculate the contribution to the gyromagnetic factor from the muon magnetic loop.
On calculating disconnected-type hadronic light-by-light scattering diagrams from lattice QCD
Hayakawa, M; Christ, N H; Izubuchi, T; Jin, L C; Lehner, C
2015-01-01
For reliable comparison of the standard model prediction to the muon g-2 with its experimental value, the hadronic light-by-light scattering (HLbL) contribution must be calculated by lattice QCD simulation. HLbL contribution has many types of disconnected-type diagrams. Here, we start with recalling the point that must be taken care of in every method to calculate them by lattice QCD, and present one concrete method called nonperturbative QED method.
Light-by-light scattering in the Lamb shift and the bound electron g factor
Czarnecki, Andrzej
2016-01-01
We compute an $\\mathcal{O}\\left(\\alpha^2(Z\\alpha)^6\\right)$ contribution to the hydrogen-atom Lamb shift arising from the light-by-light scattering. Analogous diagrams, with one atomic electric field insertion replaced by an external magnetic field, contribute to the gyromagnetic factor of the bound electron at $\\mathcal{O}\\left(\\alpha^2(Z\\alpha)^4\\right)$. We also calculate the contribution to the gyromagnetic factor from the muon magnetic loop.
Ultrafast image-based dynamic light scattering for nanoparticle sizing
Energy Technology Data Exchange (ETDEWEB)
Zhou, Wu; Zhang, Jie; Liu, Lili; Cai, Xiaoshu, E-mail: usst-caixs@163.com [Institute of Particle and Two-Phase Flow Measurement, Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering, University of Shanghai for Science and Technology, 516 Jungong Road, Shanghai 200093 (China)
2015-11-15
An ultrafast sizing method for nanoparticles is proposed, called as UIDLS (Ultrafast Image-based Dynamic Light Scattering). This method makes use of the intensity fluctuation of scattered light from nanoparticles in Brownian motion, which is similar to the conventional DLS method. The difference in the experimental system is that the scattered light by nanoparticles is received by an image sensor instead of a photomultiplier tube. A novel data processing algorithm is proposed to directly get correlation coefficient between two images at a certain time interval (from microseconds to milliseconds) by employing a two-dimensional image correlation algorithm. This coefficient has been proved to be a monotonic function of the particle diameter. Samples of standard latex particles (79/100/352/482/948 nm) were measured for validation of the proposed method. The measurement accuracy of higher than 90% was found with standard deviations less than 3%. A sample of nanosilver particle with nominal size of 20 ± 2 nm and a sample of polymethyl methacrylate emulsion with unknown size were also tested using UIDLS method. The measured results were 23.2 ± 3.0 nm and 246.1 ± 6.3 nm, respectively, which is substantially consistent with the transmission electron microscope results. Since the time for acquisition of two successive images has been reduced to less than 1 ms and the data processing time in about 10 ms, the total measuring time can be dramatically reduced from hundreds seconds to tens of milliseconds, which provides the potential for real-time and in situ nanoparticle sizing.
Nonlinear scattering in hard tissue studied with ultrashort laser pulses
Energy Technology Data Exchange (ETDEWEB)
Eichler, J. [Technische Fachhochschule Berlin, Univ. of Applied Sciences (Germany); Kim, B.M. [Yonsei Univ., Wonjoo, Kangwon-Do (Korea)
2002-07-01
The back-scattered spectrum of ultrashort laser pulses (800 nm, 0.2 ps) was studied in human dental and other hard tissues in vitro below the ablation threshold. Frequency doubled radiation (SHG), frequency tripled radiation and two-photon fluorescence were detected. The relative yield for these processes was measured for various pulse energies. The dependence of the SHG signal on probe thickness was determined in forward and back scattering geometry. SHG is sensitive to linear polarization of the incident laser radiation. SHG in human teeth was studied in vitro showing larger signals in dentin than in cementum and enamel. In carious areas no SHG signal could be detected. Possible applications of higher harmonic radiation for diagnostics and microscopy are discussed. (orig.)
Multiple scattering of light in three-dimensional photonic quasicrystals.
Ledermann, Alexandra; Wiersma, Diederik S; Wegener, Martin; von Freymann, Georg
2009-02-01
Recent experiments on three-dimensional icosahedral dielectric photonic quasicrystals have shown several unexpected features: transmitted femtosecond pulses developed a trailing "diffusive" exponential tail and the sum of (zeroth-order) transmittance and reflectance was well below unity. These experimental findings have previously been ascribed to sample imperfections. Here, we analyze these findings by using 3D periodic approximants of the ideal photonic quasicrystals. We show that the experimental observations can be explained in terms of multiple scattering of light within these structures, i.e., in terms of intrinsic rather than purely extrinsic quasicrystal properties.
Wide-field imaging through scattering media by scattered light fluorescence microscopy
Zhou, Yulan; Li, Xun
2017-08-01
To obtain images through scattering media, scattered light fluorescence (SLF) microscopy that utilizes the optical memory effect has been developed. However, the small field of view (FOV) of SLF microscopy limits its application. In this paper, we have introduced a re-modulation method to achieve wide-field imaging through scattering media by SLF microscopy. In the re-modulation method, to raster scan the focus across the object plane, the incident wavefront is re-modulated via a spatial light modulator (SLM) in the updated phase compensation calculated using the optimized iterative algorithm. Compared with the conventional optical memory effect method, the re-modulation method can greatly increase the FOV of a SLF microscope. With the phase compensation theoretically calculated, the process of updating the phase compensation of a high speed SLM is fast. The re-modulation method does not increase the imaging time. The re-modulation method is, therefore, expected to make SLF microscopy have much wider applications in biology, medicine and physiology.
HD100546 multi-epoch scattered light observations
Energy Technology Data Exchange (ETDEWEB)
Avenhaus, Henning; Quanz, Sascha P.; Meyer, Michael R. [ETH Zurich, Institute for Astronomy, Wolfgang-Pauli-Strasse 27, 8093 Zurich (Switzerland); Brittain, Sean D. [Department of Physics and Astronomy, 118 Kinard Laboratory, Clemson University, Clemson, SC 29634 (United States); Carr, John S. [Naval Research Laboratory, Code 7211, Washington, DC 20375 (United States); Najita, Joan R., E-mail: havenhaus@astro.phys.ethz.ch [National Optical Astronomy Observatory, 950 North Cherry Avenue, Tucson, AZ 85719 (United States)
2014-07-20
We present H, K{sub s}, and L' filter polarimetric differential imaging (PDI) data for the transitional disk around HD100546 obtained in 2013, together with an improved re-reduction of previously published 2006 data. We reveal the disk in polarized scattered light in all three filters, achieving an inner working angle of ∼0.''1. Additional, short-exposure observations in the H and K{sub s} filters probe the surroundings of the star down to ∼0.''03 (∼3 AU). HD100546 is fascinating because of its variety of sub-structures possibly related to forming planets in the disk, and PDI is currently the best technique for imaging them in the near-IR. For the first time ever, we detect a disk in L-band PDI data, and we constrain the outer radius of the inner hole to 14 ± 2 AU and its eccentricity to <0.133. A dark lane is detected between ∼0.''2-0.''6 AU in the front side of the disk, which is likely an effect of the scattering angle and the scattering function of the grains. We find a spiral arm in the northeast that has no obvious connection to spiral arms seen before by other authors further out in the disk, but winds are in the same direction (clockwise). The two bright scattering peaks along the semi-major axis are asymmetric, with the southeastern one being significantly brighter. This could be related to the inner companion candidate that is close to the brighter side of the disk at the time of the observations. The scattering color is close to gray between the H and K{sub s} filters ([H]–[K{sub s}] = 0.19 ± 0.11), but the scattering in the L' filter is significantly weaker ([H]–[L'] = –1.08 ± 0.35, [K{sub s}]–[L'] = –1.27 ± 0.35). We measure the position angle of the disk to be 138° ± 3°, consistent with previous observations, and we derive the dust scattering function in the H and K{sub s} filters between ∼35° and ∼130° at two different radii (30-50 and 80-110 AU) and show that
Energy Technology Data Exchange (ETDEWEB)
Alvarez-Estrada, R.F.
1979-08-01
A comprehensive review of the inverse scattering solution of certain non-linear evolution equations of physical interest in one space dimension is presented. We explain in some detail the interrelated techniques which allow to linearize exactly the following equations: (1) the Korteweg and de Vries equation; (2) the non-linear Schrodinger equation; (3) the modified Korteweg and de Vries equation; (4) the Sine-Gordon equation. We concentrate in discussing the pairs of linear operators which accomplish such an exact linearization and the solution of the associated initial value problem. The application of the method to other non-linear evolution equations is reviewed very briefly.
Coherence effects in scattering order expansion of light by atomic clouds
Rouabah, Mohamed-Taha; Bachelard, Romain; Courteille, Philippe W; Kaiser, Robin; Piovella, Nicola
2014-01-01
We interpret cooperative scattering by a collection of cold atoms as a multiple scattering process. Starting from microscopic equations describing the response of $N$ atoms to a probe light beam, we represent the total scattered field as an infinite series of multiple scattering events. As an application of the method, we obtain analytical expressions of the coherent intensity in the double scattering approximation for Gaussian density profiles. In particular, we quantify the contributions of coherent backward and forward scattering.
Coherence effects in scattering order expansion of light by atomic clouds.
Rouabah, Mohamed-Taha; Samoylova, Marina; Bachelard, Romain; Courteille, Philippe W; Kaiser, Robin; Piovella, Nicola
2014-05-01
We interpret cooperative scattering by a collection of cold atoms as a multiple-scattering process. Starting from microscopic equations describing the response of N atoms to a probe light beam, we represent the total scattered field as an infinite series of multiple-scattering events. As an application of the method, we obtain analytical expressions of the coherent intensity in the double-scattering approximation for Gaussian density profiles. In particular, we quantify the contributions of coherent backward and forward scattering.
HD100546 Multi-Epoch Scattered-Light Observations
Avenhaus, Henning; Meyer, Michael R; Brittain, Sean D; Carr, John S; Najita, Joan R
2014-01-01
We present H, Ks and L filter polarimetric differential imaging (PDI) data for the transitional disk around HD100546 obtained in 2013, together with an improved re-reduction of previously published 2006 data. We reveal the disk in polarized scattered light in all three filters, achieving an inner working angle of 0.1 arcsec. Additional, short-exposure observations in the H and Ks filter probe the surrounding of the star down to about 0.03 (about 3 AU). HD100546 is fascinating because of its variety of sub-structures possibly related to forming planets in the disk, and PDI is currently the best technique to image them in the near-IR. Our key results are: (1) For the first time ever, we detect a disk in L-band PDI data. (2) We constrain the outer radius of the inner hole to 14pm2 AU and its eccentricity to < 0.133. (3) We detect a dark lane in the front side of the disk, which is likely an effect of the scattering angle and the scattering function of the grains. (4) We find a spiral arm in the northeast whic...
Flow velocity measurement with the nonlinear acoustic wave scattering
Didenkulov, Igor; Pronchatov-Rubtsov, Nikolay
2015-10-01
A problem of noninvasive measurement of liquid flow velocity arises in many practical applications. To this end the most often approach is the use of the linear Doppler technique. The Doppler frequency shift of signal scattered from the inhomogeneities distributed in a liquid relatively to the emitted frequency is proportional to the sound frequency and velocities of inhomogeneities. In the case of very slow flow one needs to use very high frequency sound. This approach fails in media with strong sound attenuation because acoustic wave attenuation increases with frequency and there is limit in increasing sound intensity, i.e. the cavitation threshold. Another approach which is considered in this paper is based on the method using the difference frequency Doppler Effect for flows with bubbles. This method is based on simultaneous action of two high-frequency primary acoustic waves with closed frequencies on bubbles and registration of the scattered by bubbles acoustic field at the difference frequency. The use of this method is interesting since the scattered difference frequency wave has much lower attenuation in a liquid. The theoretical consideration of the method is given in the paper. The experimental examples confirming the theoretical equations, as well as the ability of the method to be applied in medical diagnostics and in technical applications on measurement of flow velocities in liquids with strong sound attenuation is described. It is shown that the Doppler spectrum form depends on bubble concentration velocity distribution in the primary acoustic beams crossing zone that allows one to measure the flow velocity distribution.
Flow velocity measurement with the nonlinear acoustic wave scattering
Energy Technology Data Exchange (ETDEWEB)
Didenkulov, Igor, E-mail: din@appl.sci-nnov.ru [Institute of Applied Physics, 46 Ulyanov str., Nizhny Novgorod, 603950 (Russian Federation); Lobachevsky State University of Nizhny Novgorod, 23 Gagarin ave., Nizhny Novgorod, 603950 (Russian Federation); Pronchatov-Rubtsov, Nikolay, E-mail: nikvas@rf.unn.ru [Lobachevsky State University of Nizhny Novgorod, 23 Gagarin ave., Nizhny Novgorod, 603950 (Russian Federation)
2015-10-28
A problem of noninvasive measurement of liquid flow velocity arises in many practical applications. To this end the most often approach is the use of the linear Doppler technique. The Doppler frequency shift of signal scattered from the inhomogeneities distributed in a liquid relatively to the emitted frequency is proportional to the sound frequency and velocities of inhomogeneities. In the case of very slow flow one needs to use very high frequency sound. This approach fails in media with strong sound attenuation because acoustic wave attenuation increases with frequency and there is limit in increasing sound intensity, i.e. the cavitation threshold. Another approach which is considered in this paper is based on the method using the difference frequency Doppler Effect for flows with bubbles. This method is based on simultaneous action of two high-frequency primary acoustic waves with closed frequencies on bubbles and registration of the scattered by bubbles acoustic field at the difference frequency. The use of this method is interesting since the scattered difference frequency wave has much lower attenuation in a liquid. The theoretical consideration of the method is given in the paper. The experimental examples confirming the theoretical equations, as well as the ability of the method to be applied in medical diagnostics and in technical applications on measurement of flow velocities in liquids with strong sound attenuation is described. It is shown that the Doppler spectrum form depends on bubble concentration velocity distribution in the primary acoustic beams crossing zone that allows one to measure the flow velocity distribution.
Nonlinear Schroedinger excitations scattering on local barrier in one dimension
Kovrizhin, D L
2001-01-01
The task on the excitations scattering of the Bose condensate under consideration on the unidimensional barrier is nontrivial one even in the case of a low barrier because the barrier itself and change in the condensate density in its vicinity play the similar important role. It is shown that if any repulsive barrier for a bare particle within the range of the waves high lengths is impermeable, than the coefficient of the delta-functional transmission for the phonons within this range strives to the unity and the barrier becomes transparent
Effects of nonlinear phase modulation on Bragg scattering in the low-conversion regime
DEFF Research Database (Denmark)
Andersen, Lasse Mejling; Cargill, D. S.; McKinstrie, C. J.
2012-01-01
In this paper, we consider the effects of nonlinear phase modulation on frequency conversion by four-wave mixing (Bragg scattering) in the low-conversion regime. We derive the Green functions for this process using the time-domain collision method, for partial collisions, in which the four fields...
Non-Linear Rheological Properties and Neutron Scattering Investigation on Dilute Ring-Linear Blends
DEFF Research Database (Denmark)
Pyckhout-Hintzen, W.; Bras, A.R.; Wischnewski, A.;
Linear and non-linear Rheology on dilute blends of polystyrene ring polymers in linear matrix is combined with Small Angle Neutron Scattering (SANS) investigations. In this way 2 different entanglement interactions become clear. After stretching the samples to different hencky strains up to 2 in ...
Effects of nonlinear phase modulation on low-conversion four-wave mixing Bragg scattering
DEFF Research Database (Denmark)
Andersen, Lasse Mejling; McKinstrie, C. J.; Rottwitt, Karsten
We consider the effects of nonlinear phase modulation (NPM) on frequency converseon by Bragg scattering. Previously we found that arbitrary mode reshaping without temporal entanglement (separability) was possible. When NPM is included, the modes are chirped and the separability is no longer compl...
The Spectrum of the Diffuse Galactic Light I: The Milky Way in Scattered Light
Brandt, Timothy D
2011-01-01
We measure the optical spectrum of the Diffuse Galactic Light--the local Milky Way in reflection--using 92,000 blank-sky spectra from the Sloan Digital Sky Survey. We correlate the SDSS optical flux density in regions of blank sky against 100 \\mu{}m intensity independently measured by the COBE and IRAS satellites, which provides a measure of the dust column density times the intensity of illuminating starlight. The spectrum of scattered light is very blue and shows a clear 4000 \\AA{} break and broad Mg b absorption. This is consistent with scattered starlight, and the continuum of the diffuse galactic light is well-reproduced by a simple radiative transfer model of the Galaxy. We also detect line emission in H\\alpha, H\\beta, [N II], and [S II], consistent with scattered light from the local interstellar medium. The strength of [N II] and [S II], combined with upper limits on [O III] and [He I], indicate a relatively soft ionizing spectrum. We find that our measurements of the diffuse galactic light can constr...
Fining of Red Wine Monitored by Multiple Light Scattering.
Ferrentino, Giovanna; Ramezani, Mohsen; Morozova, Ksenia; Hafner, Daniela; Pedri, Ulrich; Pixner, Konrad; Scampicchio, Matteo
2017-07-12
This work describes a new approach based on multiple light scattering to study red wine clarification processes. The whole spectral signal (1933 backscattering points along the length of each sample vial) were fitted by a multivariate kinetic model that was built with a three-step mechanism, implying (1) adsorption of wine colloids to fining agents, (2) aggregation into larger particles, and (3) sedimentation. Each step is characterized by a reaction rate constant. According to the first reaction, the results showed that gelatin was the most efficient fining agent, concerning the main objective, which was the clarification of the wine, and consequently the increase in its limpidity. Such a trend was also discussed in relation to the results achieved by nephelometry, total phenols, ζ-potential, color, sensory, and electronic nose analyses. Also, higher concentrations of the fining agent (from 5 to 30 g/100 L) or higher temperatures (from 10 to 20 °C) sped up the process. Finally, the advantage of using the whole spectral signal vs classical univariate approaches was demonstrated by comparing the uncertainty associated with the rate constants of the proposed kinetic model. Overall, multiple light scattering technique showed a great potential for studying fining processes compared to classical univariate approaches.
Flow speed measurement using two-point collective light scattering
Energy Technology Data Exchange (ETDEWEB)
Heinemeier, N.P
1998-09-01
Measurements of turbulence in plasmas and fluids using the technique of collective light scattering have always been plagued by very poor spatial resolution. In 1994, a novel two-point collective light scattering system for the measurement of transport in a fusion plasma was proposed. This diagnostic method was design for a great improvement of the spatial resolution, without sacrificing accuracy in the velocity measurement. The system was installed at the W7-AS steallartor in Garching, Germany, in 1996, and has been operating since. This master thesis is an investigation of the possible application of this new method to the measurement of flow speeds in normal fluids, in particular air, although the results presented in this work have significance for the plasma measurements as well. The main goal of the project was the experimental verification of previous theoretical predictions. However, the theoretical considerations presented in the thesis show that the method can only be hoped to work for flows that are almost laminar and shearless, which makes it of very small practical interest. Furthermore, this result also implies that the diagnostic at W7-AS cannot be expected to give the results originally hoped for. (au) 1 tab., 51 ills., 29 refs.
Lysozyme Aggregation and Fibrillation Monitored by Dynamic Light Scattering
Nemzer, Louis; Flanders, Bret; Schmit, Jeremy; Sorensen, Christopher
2012-02-01
The aggregation of amyloidogenic proteins provides a rich phase space with significant biomedical implications, including a link with several age-related diseases. We employed dynamic light scattering to monitor the aggregation of lysozyme, a model protein, from a monomeric state until the formation of micron-sized fibrils. For an aqueous lysozyme solution buffered at pH 2, the auto-correlation function of the scattered light intensity was found to be well-fit by a single exponential function with decay time τ = 1/(2Dq^2) = 0.25 ms, which corresponds to a mean hydrodynamic radius (RH) of 2.2 nm, very likely generated by monomers. Ethanol (4% v/v final concentration) induced a partial unfolding, to RH = 4.6 nm. The subsequent addition of 70 mM KCl was found to shrink the size back to RH = 2.5 nm, as expected when a denatured protein refolds due to partial screening of the intramolecular repulsion. However, further aggregation was not observed. At pH 4, using a low-salt acetate buffer, more ethanol (10% v/v) was required to initiate unfolding, but once it occurred, larger aggregates formed. These results are consistent with the model that partial unfolding, which exposes beta-motif secondary structure, is a prerequisite for aggregation and fibrillation, but the aggregation fate depends on the protein charge state (pH) and screening (salt concentration).
Scattered H-alpha light from Galactic dust clouds
Mattila, K; Lehtinen, K
2006-01-01
Bright emission nebulae, or HII regions, around hot stars are readily seen in H-alpha light. However, the all-pervasive faint H-alpha emission has only recently been detected and mapped over the whole sky. Mostly the H-alpha emission observed along a line of sight is produced by ionised gas in situ. There are, however, cases where all or most of the H-alpha radiation is due to scattering by electrons or dust particles which are illuminated by an H-alpha emitting source off the line of sight. Here we demonstrate that diffuse, translucent and dark dust clouds at high galactic latitudes are in many cases observed to have an excess of diffuse H-alpha surface brightness, i.e. they are brighter than the surrounding sky. We show that the majority of this excess surface brightness can be understood as light scattered off the interstellar dust grains. The source of incident photons is the general Galactic H-alpha background radiation impinging on the dust clouds from all over the sky.
THEORETICAL-MODEL FOR THE SCATTERING OF LIGHT BY DENTIN AND COMPARISON WITH MEASUREMENTS
ZIJP, [No Value; TENBOSCH, JJ
1993-01-01
A theoretical model of the scattering of light by dentin is presented. The model that results is a superposition of several scattering contributions, i.e., scattering by mineral crystals, collagen fibrils, and dentinal tubules. These tubules are oriented so that they cause an asymmetrical scattering
Fractal scattering of Gaussian solitons in directional couplers with logarithmic nonlinearities
Energy Technology Data Exchange (ETDEWEB)
Teixeira, Rafael M.P.; Cardoso, Wesley B., E-mail: wesleybcardoso@gmail.com
2016-08-12
In this paper we study the interaction of Gaussian solitons in a dispersive and nonlinear media with log-law nonlinearity. The model is described by the coupled logarithmic nonlinear Schrödinger equations, which is a nonintegrable system that allows the observation of a very rich scenario in the collision patterns. By employing a variational approach and direct numerical simulations, we observe a fractal-scattering phenomenon from the exit velocities of each soliton as a function of the input velocities. Furthermore, we introduce a linearization model to identify the position of the reflection/transmission window that emerges within the chaotic region. This enables us the possibility of controlling the scattering of solitons as well as the lifetime of bound states. - Highlights: • We study the interaction of Gaussian solitons in a system with log-law nonlinearity. • The model is described by the coupled logarithmic nonlinear Schrödinger equations. • We observe a fractal-scattering phenomenon of the solitons.
Modeling diffuse reflectance measurements of light scattered by layered tissues
Rohde, Shelley B.
In this dissertation, we first present a model for the diffuse reflectance due to a continuous beam incident normally on a half space composed of a uniform scattering and absorbing medium. This model is the result of an asymptotic analysis of the radiative transport equation for strong scattering, weak absorption and a defined beam width. Through comparison with the diffuse reflectance computed using the numerical solution of the radiative transport equation, we show that this diffuse reflectance model gives results that are accurate for small source-detector separation distances. We then present an explicit model for the diffuse reflectance due to a collimated beam of light incident normally on layered tissues. This model is derived using the corrected diffusion approximation applied to a layered medium, and it takes the form of a convolution with an explicit kernel and the incident beam profile. This model corrects the standard diffusion approximation over all source-detector separation distances provided the beam is sufficiently wide compared to the scattering mean-free path. We validate this model through comparison with Monte Carlo simulations. Then we use this model to estimate the optical properties of an epithelial layer from Monte Carlo simulation data. Using measurements at small source-detector separations and this model, we are able to estimate the absorption coefficient, scattering coefficient and anisotropy factor of epithelial tissues efficiently with reasonable accuracy. Finally, we present an extension of the corrected diffusion approximation for an obliquely incident beam. This model is formed through a Fourier Series representation in the azimuthal angle which allows us to exhibit the break in axisymmetry when combined with the previous analysis. We validate this model with Monte Carlo simulations. This model can also be written in the form of a convolution of an explicit kernel with the incident beam profile. Additionally, it can be used to
Chiral Huygens metasurfaces for nonlinear structuring of linearly polarized light
Lesina, A Calà; Ramunno, L
2016-01-01
We report on a chiral nanostructure, which we term a "butterfly nanoantenna," that, when used in a metasurface, allows the direct conversion of a linearly polarized beam into a nonlinear optical far-field of arbitrary complexity. The butterfly nanoantenna exhibits field enhancement in its gap for every incident linear polarization, which can be exploited to drive nonlinear optical emitters within the gap, for the structuring of light within a frequency range not accessible by linear plasmonics. As the polarization, phase and amplitude of the field in the gap are highly controlled, nonlinear emitters within the gap behave as an idealized Huygens source. A general framework is thereby proposed wherein the butterfly nanoantennas can be arranged on a surface to produce a highly structured far-field nonlinear optical beam with high purity. A third harmonic Laguerre-Gauss beam carrying an optical orbital angular momentum of 41 is demonstrated as an example, through large-scale simulations on a high-performance comp...
Stimulated Raman Scattering and Nonlinear Focusing of High-Power Laser Beams Propagating in Water
Hafizi, B; Penano, J R; Gordon, D F; Jones, T G; Helle, M H; Kaganovich, D
2015-01-01
The physical processes associated with propagation of a high-power (power > critical power for self-focusing) laser beam in water include nonlinear focusing, stimulated Raman scattering (SRS), optical breakdown and plasma formation. The interplay between nonlinear focusing and SRS is analyzed for cases where a significant portion of the pump power is channeled into the Stokes wave. Propagation simulations and an analytical model demonstrate that the Stokes wave can re-focus the pump wave after the power in the latter falls below the critical power. It is shown that this novel focusing mechanism is distinct from cross-phase focusing. While discussed here in the context of propagation in water, the gain-focusing phenomenon is general to any medium supporting nonlinear focusing and stimulated forward Raman scattering.
Scattering of time-harmonic elastic waves by an elastic inclusion with quadratic nonlinearity.
Tang, Guangxin; Jacobs, Laurence J; Qu, Jianmin
2012-04-01
This paper considers the scattering of a plane, time-harmonic wave by an inclusion with heterogeneous nonlinear elastic properties embedded in an otherwise homogeneous linear elastic solid. When the inclusion and the surrounding matrix are both isotropic, the scattered second harmonic fields are obtained in terms of the Green's function of the surrounding medium. It is found that the second harmonic fields depend on two independent acoustic nonlinearity parameters related to the third order elastic constants. Solutions are also obtained when these two acoustic nonlinearity parameters are given as spatially random functions. An inverse procedure is developed to obtain the statistics of these two random functions from the measured forward and backscattered second harmonic fields.
Zhao, Ming; Zhang, Han; Li, Yu; Ashok, Amit; Liang, Rongguang; Zhou, Weibin; Peng, Leilei
2014-01-01
In vivo fluorescent cellular imaging of deep internal organs is highly challenging, because the excitation needs to penetrate through strong scattering tissue and the emission signal is degraded significantly by photon diffusion induced by tissue-scattering. We report that by combining two-photon Bessel light-sheet microscopy with nonlinear structured illumination microscopy (SIM), live samples up to 600 microns wide can be imaged by light-sheet microscopy with 500 microns penetration depth, and diffused background in deep tissue light-sheet imaging can be reduced to obtain clear images at cellular resolution in depth beyond 200 microns. We demonstrate in vivo two-color imaging of pronephric glomeruli and vasculature of zebrafish kidney, whose cellular structures located at the center of the fish body are revealed in high clarity by two-color two-photon Bessel light-sheet SIM. PMID:24876996
Zhao, Ming; Zhang, Han; Li, Yu; Ashok, Amit; Liang, Rongguang; Zhou, Weibin; Peng, Leilei
2014-05-01
In vivo fluorescent cellular imaging of deep internal organs is highly challenging, because the excitation needs to penetrate through strong scattering tissue and the emission signal is degraded significantly by photon diffusion induced by tissue-scattering. We report that by combining two-photon Bessel light-sheet microscopy with nonlinear structured illumination microscopy (SIM), live samples up to 600 microns wide can be imaged by light-sheet microscopy with 500 microns penetration depth, and diffused background in deep tissue light-sheet imaging can be reduced to obtain clear images at cellular resolution in depth beyond 200 microns. We demonstrate in vivo two-color imaging of pronephric glomeruli and vasculature of zebrafish kidney, whose cellular structures located at the center of the fish body are revealed in high clarity by two-color two-photon Bessel light-sheet SIM.
A Time Marching Scheme for Solving Volume Integral Equations on Nonlinear Scatterers
Bagci, Hakan
2015-01-07
Transient electromagnetic field interactions on inhomogeneous penetrable scatterers can be analyzed by solving time domain volume integral equations (TDVIEs). TDVIEs are oftentimes solved using marchingon-in-time (MOT) schemes. Unlike finite difference and finite element schemes, MOT-TDVIE solvers require discretization of only the scatterers, do not call for artificial absorbing boundary conditions, and are more robust to numerical phase dispersion. On the other hand, their computational cost is high, they suffer from late-time instabilities, and their implicit nature makes incorporation of nonlinear constitutive relations more difficult. Development of plane-wave time-domain (PWTD) and FFT-based schemes has significantly reduced the computational cost of the MOT-TDVIE solvers. Additionally, latetime instability problem has been alleviated for all practical purposes with the development of accurate integration schemes and specially designed temporal basis functions. Addressing the third challenge is the topic of this presentation. I will talk about an explicit MOT scheme developed for solving the TDVIE on scatterers with nonlinear material properties. The proposed scheme separately discretizes the TDVIE and the nonlinear constitutive relation between electric field intensity and flux density. The unknown field intensity and flux density are expanded using half and full Schaubert-Wilton-Glisson (SWG) basis functions in space and polynomial temporal interpolators in time. The resulting coupled system of the discretized TDVIE and constitutive relation is integrated in time using an explicit P E(CE) m scheme to yield the unknown expansion coefficients. Explicitness of time marching allows for straightforward incorporation of the nonlinearity as a function evaluation on the right hand side of the coupled system of equations. Consequently, the resulting MOT scheme does not call for a Newton-like nonlinear solver. Numerical examples, which demonstrate the applicability
Non-linear analysis in Light Water Reactor design
Energy Technology Data Exchange (ETDEWEB)
Rashid, Y.R.; Sharabi, M.N.; Nickell, R.E.; Esztergar, E.P.; Jones, J.W.
1980-03-01
The results obtained from a scoping study sponsored by the US Department of Energy (DOE) under the Light Water Reactor (LWR) Safety Technology Program at Sandia National Laboratories are presented. Basically, this project calls for the examination of the hypothesis that the use of nonlinear analysis methods in the design of LWR systems and components of interest include such items as: the reactor vessel, vessel internals, nozzles and penetrations, component support structures, and containment structures. Piping systems are excluded because they are being addressed by a separate study. Essentially, the findings were that nonlinear analysis methods are beneficial to LWR design from a technical point of view. However, the costs needed to implement these methods are the roadblock to readily adopting them. In this sense, a cost-benefit type of analysis must be made on the various topics identified by these studies and priorities must be established. This document is the complete report by ANATECH International Corporation.
Polyelectrolyte Conformation, Interactions and Hydrodynamics as Studied by Light Scattering.
Ghosh, Snehasish
Polyelectrolyte conformation, interactions and hydrodynamics show a marked dependence on the ionic strength (C_{rm s}) of the medium, the concentration (C_{rm p}) of the polymer itself and their charge density (xi). The apparent electrostatic persistence length obtained from static light scattering varied approximately as the inverse square root of C _{rm s} for highly pure, high molecular weight hyaluronate (HA) as well as for variably ionized acrylamide/sodium acrylate copolymers (NaPAA), and linearly with xi. The experimental values of persistence length and second virial coefficient (A_2) are compared to predictions from theories based on the Debye-Huckel approximation for the Poisson-Boltzmann equation and on excluded-volume. Although the mean square radius of gyration () depended strongly on C _{rm s}. decreasing with increasing C_{rm s} for both HA and NaPAA indicating clear evidence of polyion expansion, dynamic light scattering values of the translational diffusion coefficient (D) remains constant when extrapolated to infinite polymer concentration for both the polymers. The behavior of D is compared to predictions from coupled mode theory in the linear limit. The effects of NaOH on the conformations, interactions, diffusion and hydrolysis rates of HA are characterized in detail using static, dynamic and time-dependent light scattering supplemented by size exclusion chromatography (SEC). For the HA , A_2 and the hydrolysis rates all resemble superposing titration curves, while the D remains independent of both the concentration of NaOH, and the contraction of . The indication is that the interactions, conformations and the hydrolysis rates are all controlled by the titration of the HA hydroxyl groups by the NaOH to yield -O ^-, which (i) destroys single strand hydrogen bonds, leading to de-stiffening and contraction of the HA coil and a large decrease in intermolecular interaction, and (ii) slowly depolymerizes HA. The experimental results of HA
A schlieren method for ultra-low angle light scattering measurements
Brogioli, D; Giglio, M; Giglio, Marzio
2003-01-01
We describe a self calibrating optical technique that allows to perform absolute measurements of scattering cross sections for the light scattered at extremely small angles. Very good performances are obtained by using a very simple optical layout similar to that used for the schlieren method, a technique traditionally used for mapping local refraction index changes. The scattered intensity distribution is recovered by a statistical analysis of the random interference of the light scattered in a half-plane of the scattering wave vectors and the main transmitted beam. High quality data can be obtained by proper statistical accumulation of scattered intensity frames, and the static stray light contributions can be eliminated rigorously. The potentialities of the method are tested in a scattering experiment from non equilibrium fluctuations during a free diffusion experiment. Contributions of light scattered from length scales as long as Lambda=1 mm can be accurately determined.
Simplifying the calculation of light scattering properties for black carbon fractal aggregates
Smith, A. J. A.; Grainger, R. G.
2014-02-01
Black carbon fractal aggregates have complicated shapes that make the calculation of their optical properties particularly computationally expensive. Here, a method is presented to estimate fractal aggregate light scattering properties by optimising simplified models to full light scattering calculations. It is found that there are no possible spherical models (at any size or refractive index) that well represent the light scattering in the visible, or near-thermal infrared. As such, parameterisations of the light scattering as a function of the number of aggregate particles is presented as the most pragmatic choice for modelling distributions of black carbon when the large computational overheads of rigorous scattering calculations cannot be justified. This parameterisation can be analytically integrated to provide light scattering properties for log-normal distributions of black carbon fractal aggregates and return extinction cross-sections with 0.1% accuracy for typical black carbon size distributions. Scattering cross-sections and the asymmetry parameter can be obtained to within 3%.
Simplifying the calculation of light scattering properties for black carbon fractal aggregates
Directory of Open Access Journals (Sweden)
A. J. A. Smith
2014-08-01
Full Text Available Black carbon fractal aggregates have complicated shapes that make the calculation of their optical properties particularly computationally expensive. Here, a method is presented to estimate fractal aggregate light scattering properties by optimising simplified models to full light scattering calculations. It is found that there are no possible spherical models (at any size or refractive index that well represent the light scattering in the visible or near-thermal infrared. As such, parameterisations of the light scattering as a function of the number of aggregate particles is presented as the most pragmatic choice for modelling distributions of black carbon when the large computational overheads of rigorous scattering calculations cannot be justified. This parameterisation can be analytically integrated to provide light scattering properties for lognormal distributions of black carbon fractal aggregates and return extinction cross sections with 0.1% accuracy for typical black carbon size distributions. Scattering cross sections and the asymmetry parameter can be obtained to within 3%.
The Effects of Scattered Light from Optical Components on Visual Function
2016-02-01
measures light scatter in the human eye (intraocular scatter) over a region from ~5° - 10° from the optical axis, or at an average scatter angle of...contrast sensitivity were measured in twelve subjects without and with eight different optical materials (OM) positioned in front of their right eye ... measure light scatter with and without an optical component in front of the eye and then calculating the difference, may provide data to derive a measure
Pandey, Ravindra; Ghosh, Sampa; Mukhopadhyay, S; Ramasesha, S; Das, Puspendu K
2011-01-28
We report large quadratic nonlinearity in a series of 1:1 molecular complexes between methyl substituted benzene donors and quinone acceptors in solution. The first hyperpolarizability, β(HRS), which is very small for the individual components, becomes large by intermolecular charge transfer (CT) interaction between the donor and the acceptor in the complex. In addition, we have investigated the geometry of these CT complexes in solution using polarization resolved hyper-Rayleigh scattering (HRS). Using linearly (electric field vector along X direction) and circularly polarized incident light, respectively, we have measured two macroscopic depolarization ratios D=I(2ω,X,X)/I(2ω,Z,X) and D(')=I(2ω,X,C)/I(2ω,Z,C) in the laboratory fixed XYZ frame by detecting the second harmonic scattered light in a polarization resolved fashion. The experimentally obtained first hyperpolarizability, β(HRS), and the value of macroscopic depolarization ratios, D and D('), are then matched with the theoretically deduced values from single and double configuration interaction calculations performed using the Zerner's intermediate neglect of differential overlap self-consistent reaction field technique. In solution, since several geometries are possible, we have carried out calculations by rotating the acceptor moiety around three different axes keeping the donor molecule fixed at an optimized geometry. These rotations give us the theoretical β(HRS), D and D(') values as a function of the geometry of the complex. The calculated β(HRS), D, and D(') values that closely match with the experimental values, give the dominant equilibrium geometry in solution. All the CT complexes between methyl benzenes and chloranil or 1,2-dichloro-4,5-dicyano-p-benzoquinone investigated here are found to have a slipped parallel stacking of the donors and the acceptors. Furthermore, the geometries are staggered and in some pairs, a twist angle as high as 30° is observed. Thus, we have demonstrated in
Light scattering by planetary-regolith analog samples: computational results
Väisänen, Timo; Markkanen, Johannes; Hadamcik, Edith; Levasseur-Regourd, Anny-Chantal; Lasue, Jeremie; Blum, Jürgen; Penttilä, Antti; Muinonen, Karri
2017-04-01
We compute light scattering by a planetary-regolith analog surface. The corresponding experimental work is from Hadamcik et al. [1] with the PROGRA2-surf [2] device measuring the polarization of dust particles. The analog samples are low density (volume fraction 0.15 ± 0.03) agglomerates produced by random ballistic deposition of almost equisized silica spheres (refractive index n=1.5 and diameter 1.45 ± 0.06 µm). Computations are carried out with the recently developed codes entitled Radiative Transfer with Reciprocal Transactions (R2T2) and Radiative Transfer Coherent Backscattering with incoherent interactions (RT-CB-ic). Both codes incorporate the so-called incoherent treatment which enhances the applicability of the radiative transfer as shown by Muinonen et al. [3]. As a preliminary result, we have computed scattering from a large spherical medium with the RT-CB-ic using equal-sized particles with diameters of 1.45 microns. The preliminary results have shown that the qualitative characteristics are similar for the computed and measured intensity and polarization curves but that there are still deviations between the characteristics. We plan to remove the deviations by incorporating a size distribution of particles (1.45 ± 0.02 microns) and detailed information about the volume density profile within the analog surface. Acknowledgments: We acknowledge the ERC Advanced Grant no. 320773 entitled Scattering and Absorption of Electromagnetic Waves in Particulate Media (SAEMPL). Computational resources were provided by CSC - IT Centre for Science Ltd, Finland. References: [1] Hadamcik E. et al. (2007), JQSRT, 106, 74-89 [2] Levasseur-Regourd A.C. et al. (2015), Polarimetry of stars and planetary systems, CUP, 61-80 [3] Muinonen K. et al. (2016), extended abstract for EMTS.
DEFF Research Database (Denmark)
Nysteen, Anders; McCutcheon, Dara; Mørk, Jesper
2015-01-01
We analytically treat the scattering of two counterpropagating photons on a two-level emitter embedded in an optical waveguide. We find that the nonlinearity of the emitter can give rise to significant pulse-dependent directional correlations in the scattered photonic state, which could...... be quantified via a reduction in coincidence clicks in a Hong–Ou–Mandel measurement setup, analogous to a linear beam splitter. Changes to the spectra and phase of the scattered photons, however, would lead to reduced interference with other photons when implemented in a larger optical circuit. We introduce...... suitable fidelity measures which account for these changes and find that high values can still be achieved even when accounting for all properties of the scattered photonic state....
Detection of circular polarization in light scattered from photosynthetic microbes
Sparks, William B; Germer, Thomas A; Chen, Feng; DasSarma, Shiladitya; DasSarma, Priya; Robb, Frank T; Manset, Nadine; Kolokolova, Ludmilla; Reid, Neill; Macchetto, F Duccio; Martin, William; 10.1073/pnas.0810215106
2009-01-01
The identification of a universal biosignature that could be sensed remotely is critical to the prospects for success in the search for life elsewhere in the universe. A candidate universal biosignature is homochirality, which is likely to be a generic property of all biochemical life. Due to the optical activity of chiral molecules, it has been hypothesized that this unique characteristic may provide a suitable remote sensing probe using circular polarization spectroscopy. Here, we report the detection of circular polarization in light scattered by photosynthetic microbes. We show that the circular polarization appears to arise from circular dichroism of the strong electronic transitions of photosynthetic absorption bands. We conclude that circular polarization spectroscopy could provide a powerful remote sensing technique for generic life searches.
Brillouin light scattering studies of 2D magnonic crystals
Tacchi, S.; Gubbiotti, G.; Madami, M.; Carlotti, G.
2017-02-01
Magnonic crystals, materials with periodic modulation of their magnetic properties, represent the magnetic counterpart of photonic, phononic and plasmonic crystals, and have been largely investigated in recent years because of the possibility of using spin waves as a new means for carrying and processing information over a very large frequency bandwidth. Here, we review recent Brillouin light scattering studies of 2D magnonic crystals consisting of single- and bi-component arrays of interacting magnetic dots or antidot lattices. In particular, we discuss the principal properties of the magnonic band diagram of such systems, with emphasis given to its dependence on both magnetic and the geometrical parameters. Thanks to the possibility of tailoring their band structure by means of several degrees of freedom, planar magnonic crystals offer a good opportunity to design an innovative class of nanoscale microwave devices.
Remnant lipoprotein size distribution profiling via dynamic light scattering analysis.
Chandra, Richa; Mellis, Birgit; Garza, Kyana; Hameed, Samee A; Jurica, James M; Hernandez, Ana V; Nguyen, Mia N; Mittal, Chandra K
2016-11-01
Remnant lipoproteins (RLP) are a metabolically derived subpopulation of triglyceride-rich lipoproteins (TRL) in human blood that are involved in the metabolism of dietary fats or triglycerides. RLP, the smaller and denser variants of TRL particles, are strongly correlated with cardiovascular disease (CVD) and were listed as an emerging atherogenic risk factor by the AHA in 2001. Varying analytical techniques used in clinical studies in the size determination of RLP contribute to conflicting hypotheses in regard to whether larger or smaller RLP particles contribute to CVD progression, though multiple pathways may exist. We demonstrated a unique combinatorial bioanalytical approach involving the preparative immunoseparation of RLP, and dynamic light scattering for size distribution analysis. This is a new facile and robust methodology for the size distribution analysis of RLP that in conjunction with clinical studies may reveal the mechanisms by which RLP cause CVD progression. Copyright © 2016 Elsevier B.V. All rights reserved.
LIGHT SCATTERING OF POLYSACCHARIDE FROM LACQUER IN AQUEOUS SOLUTION
Institute of Scientific and Technical Information of China (English)
ZHANG Lina; DU Yumin; KUMANOTANI JU
1989-01-01
The polysaccharide having weight-average molecular weight Mw= 1. 09 × 105 , isolated from the sap of lac trees ( Vietnam ), was separated into 12 fractions by aqueous-phase preparative gel permeation chromatography. The molecular weights and molecular weight distributions of the fractions were measured in aqueous 0.08M KCl/0.01 M NaAc and 0.4M KCl/0.05M NaAc at pH = 7.6 by light scattering, viscometry and gel permeation chromatography. The Mark-Houwink equation in aqueous 0.08M KCl/0.01M NaAc at30 ℃ was found to be [ η] = 2.28 ×10-2 M0.52w ( cm3/g ), which indicated the polysaccharide chain in the aqueous solution to be a spherical random coil.
Elastic scattering, fusion, and breakup of light exotic nuclei
Energy Technology Data Exchange (ETDEWEB)
Kolata, J.J. [University of Notre Dame, Physics Department, Notre Dame, IN (United States); Guimaraes, V. [Universidade de Sao Paulo, Instituto de Fisica, Sao Paulo, SP (Brazil); Aguilera, E.F. [Instituto Nacional de Investigaciones Nucleares, Departamento de Aceleradores, Mexico, Distrito Federal (Mexico)
2016-05-15
The present status of fusion reactions involving light (A< 20) radioactive projectiles at energies around the Coulomb barrier (E<10 MeV per nucleon) is reviewed, emphasizing measurements made within the last decade. Data on elastic scattering (providing total reaction cross section information) and breakup channels for the involved systems, demonstrating the relationship between these and the fusion channel, are also reviewed. Similarities and differences in the behavior of fusion and total reaction cross section data concerning halo nuclei, weakly-bound but less exotic projectiles, and strongly-bound systems are discussed. One difference in the behavior of fusion excitation functions near the Coulomb barrier seems to emerge between neutron-halo and proton-halo systems. The role of charge has been investigated by comparing the fusion excitation functions, properly scaled, for different neutron- and proton-rich systems. Possible physical explanations for the observed differences are also reviewed. (orig.)
2D Static Light Scattering for Dairy Based Applications
DEFF Research Database (Denmark)
Skytte, Jacob Lercke
Throughout this thesis we investigate a recently introduced optical technique denoted 2D static light scattering (2DSLS). The technique is remote sensing, non-invasive, highly flexible, and appears to be well suited for in-line process control. Moreover, the output signal contains contributions......, this specific process control can be highly beneficial. To provide suitable reference measures on the actual microstructure, we investigate how to quantify micrographs of yogurts objectively. We provide a comparative study, that includes a broad range of different image texture descriptors....... from several different optical phenomena, which can be utilised to provide information on chemical composition and underlying microstructure of an investigated sample. The main goal of this thesis is to provide an exploratory study of the 2DSLS technique in relation to dairy based applications...
Multifractal analysis of light scattering-intensity fluctuations
Shayeganfar, F.; Jabbari-Farouji, S.; Movahed, M. Sadegh; Jafari, G. R.; Tabar, M. Reza Rahimi
2009-12-01
We provide a simple interpretation of non-Gaussian nature of the light scattering-intensity fluctuations from an aging colloidal suspension of Laponite using the multiplicative cascade model, Markovian method, and volatility correlations. The cascade model and Markovian method enable us to reproduce most of recent empirical findings: long-range volatility correlations and non-Gaussian statistics of intensity fluctuations. We provide evidence that the intensity increments Δx(τ)=I(t+τ)-I(t) , upon different delay time scales τ , can be described as a Markovian process evolving in τ . Thus, the τ dependence of the probability density function p(Δx,τ) on the delay time scale τ can be described by a Fokker-Planck equation. We also demonstrate how drift and diffusion coefficients in the Fokker-Planck equation can be estimated directly from the data.
Evaluation of urine culture screening by light-scatter photometry
Energy Technology Data Exchange (ETDEWEB)
Hale, D.C.; Thrupp, L.D.; Matsen, J.M.
1981-08-01
Urine screening for bacteriuria by light-scatter photometry (Autobac) was evaluated for accuracy and compared with a colony count by the calibrated loop method. Incubation time, inoculum size, precision, and interference of particulate matter were evaluated in an effort to standardize the screening procedure. Results showed that urines could be accurately screened for Enterobacteriaceae by inoculating a single Autobac cuvette chamber with 0.1 or 0.2 ml of urine and determining the voltage change after four hours. A change of greater than or equal to 0.2 units indicates significant bacteriuria. Decreased accuracy was noted for urines having greater than 10(5) cfu/ml of Pseudomonas species or gram-positive cocci, possibly because these organisms grow more slowly.
Manipulating scattering of ultracold atoms with light-induced dissipation
Lemeshko, Mikhail
2013-01-01
Recently it has been shown that pairs of atoms can form metastable bonds due to non-conservative forces induced by dissipation [Lemeshko&Weimer, Nature Comm. 4, 2230 (2013)]. Here we study the dynamics of interaction-induced coherent population trapping - the process responsible for the formation of dissipatively bound molecules. We derive the effective dissipative potentials induced between ultracold atoms by laser light, and study the time evolution of the scattering states. We demonstrate that binding occurs on short timescales of ~10 microseconds, even if the initial kinetic energy of the atoms significantly exceeds the depth of the dissipative potential. Dissipatively-bound molecules with preordained bond lengths and vibrational wavefunctions can be created and detected in current experiments with ultracold atoms.
Passivated gel electrophoresis of charged nanospheres by light-scattering video tracking.
Zhu, Xiaoming; Mason, Thomas G
2014-08-15
Gel electrophoresis (gel-EP) has been used for decades to separate charged biopolymers, such as DNA, RNA, and proteins, yet propagation of other charged colloidal objects, such as nanoparticles, during gel-EP has been studied comparatively little. Simply introducing anionic nanoparticles, such as sulfate-stabilized polystyrene nanospheres, in standard large-pore agarose gels commonly used for biomolecules does not automatically ensure propagation or size-separation because attractive interactions can exist between the gel and the nanoparticles. Whereas altering the surfaces of the nanoparticles is a possible solution, here, by contrast, we show that treating a common type I-A low-electroendoosmosis agarose gel with a passivation agent, such as poly-(ethyleneglycol), enables charged nanoparticles to propagate through large-pore passivated gels in a highly reproducible manner. Moreover, by taking advantage of the significant optical scattering from the nanoparticles, which is not easily measurable for biopolymers, relative to scattering from the gel, we perform real-time, light-scattering, video-tracking gel-EP. Continuous optical measurements of the propagation of bands of uniformly sized nanospheres in passivated gels provides the propagation distance, L, and velocity, v, as a function of time for different sphere radii, electric field strengths, gel concentrations, and passivation agent concentrations. The steady-state particle velocities vary linearly with applied electric field strength, E, for small E, but these velocities become non-linear for larger E, suggesting that strongly driven nanoparticles can become elastically trapped in the smaller pores of the gel, which act like blind holes, in a manner that thermal fluctuations cannot overcome. Based on this assumption, we introduce a simple model that fits the measured v(E) in both linear and non-linear regimes over a relevant range of applied voltages. Copyright © 2014 Elsevier Inc. All rights reserved.
Bryukvina, L. I.; Pestryakov, E. V.; Kirpichnikov, A. V.; Martynovich, E. F.
2014-11-01
Modification of sodium fluoride crystal lattice by means of femtosecond laser pulses with λmax=800 nm, energy 0.5 mJ, duration 30 fs and repetition rate 1 kHz has been considered in the paper. Effective formation of simple and complex aggregate color centers and light scattering nanodefects in the channel of a laser beam in NaF crystal have been shown for the first time. Dependences of color centers concentration on the distance between the channel center and its periphery and along the channel have been presented. Influence of external focusing on color centers creation has been revealed. Explanations of the observed phenomena have been presented on the basis of nonlinear processes taking place under the effect of high-intensity femtosecond pulses.
Power-Law Behavior in Signal Scattering Process in Vertical Granular Chain with Light Impurities
Institute of Scientific and Technical Information of China (English)
XU Ai-Guo
2001-01-01
We investigate the scattering process of impulse in vertical granular chain with light impurities. When the perturbation is weak, the quantities describing the reflection rate exhibit power-law behavior with the impurity depth. The exponent is nearly independent of vi. When the perturbation is very strong, the vertical chain shows similar behavior to that of the horizontal chain, so the exponent is nearly zero. Our numerical investigation begins from the weak perturbation region and extends to the nonlinear region and found a peak of the exponent. The difficulty in extending the numerical investigation to a stronger perturbation region is analyzed.PACS numbers: 45.70.-n, 43.25.+y, 46.40.Cd
Cooperative resonances in light scattering from two-dimensional atomic arrays
Shahmoon, Ephraim; Lukin, Mikhail D; Yelin, Susanne F
2016-01-01
We consider light scattering off a two-dimensional (2D) dipolar array and show how it can be tailored by properly choosing the lattice constant of the order of the incident wavelength. In particular, we demonstrate that such arrays can operate as nearly perfect mirrors for a wide range of incident angles and frequencies close to the individual atomic resonance. These results can be understood in terms of the cooperative resonances of the surface modes supported by the 2D array. Experimental realizations are discussed, using ultracold arrays of trapped atoms and excitons in 2D semiconductor materials, as well as potential applications ranging from atomically thin metasurfaces to single photon nonlinear optics and nanomechanics.
Chen, Xiang-Jun; Lam, Wa Kun
2004-06-01
An inverse scattering transform for the derivative nonlinear Schrödinger equation with nonvanishing boundary conditions is derived by introducing an affine parameter to avoid constructing Riemann sheets. A one-soliton solution simpler than that in the literature is obtained, which is a breather and degenerates to a bright or dark soliton as the discrete eigenvalue becomes purely imaginary. The solution is mapped to that of the modified nonlinear Schrödinger equation by a gaugelike transformation, predicting some sub-picosecond solitons in optical fibers.
Nonlinear Propagation of Coupling Optical Pulse under Compton Scattering in Laser Medium
Institute of Scientific and Technical Information of China (English)
HAO Dong-shan; ZHANG Xiao-fu
2006-01-01
After considering Kerr nonlinear effect,group velocity dispersion of host and gain distribution of active particle in laser amplifying medium,a basic equation describing propagation of the coupling optical pulse under the multi-photon nonlinear Compton scattering in the laser amplifying medium has been deduced. Besides,the profile and power spectrum of a picosecond-level super-Gaussian coupling pulse in the laser amplifying medium have been discussed when its central frequency coincides with the gain peak frequency of the laser amplifying medium.
Scattering of light by Gaussian-correlated quasi-homogeneous anisotropic media.
Du, Xinyue; Zhao, Daomu
2010-02-01
We investigate the case when light is scattered by Gaussian-correlated, quasi-homogeneous, anisotropic media. The analytical expression for the cross-spectral density function of the scattered field that is produced by scattering of a polychromatic plane wave incident upon a Gaussian-correlated, quasi-homogeneous, anisotropic medium is derived by use of a tensor method. Numerical examples are given to illustrate the normalized spectral density and the spectral degree of coherence of the field scattered by the anisotropic scatterer in contrast with that scattered by the isotropic scatterer.
Buried Object Detection by an Inexact Newton Method Applied to Nonlinear Inverse Scattering
Directory of Open Access Journals (Sweden)
Matteo Pastorino
2012-01-01
Full Text Available An approach to reconstruct buried objects is proposed. It is based on the integral equations of the electromagnetic inverse scattering problem, written in terms of the Green’s function for half-space geometries. The full nonlinearity of the problem is exploited in order to inspect strong scatterers. After discretization of the continuous model, the resulting equations are solved in a regularization sense by means of a two-step inexact Newton algorithm. The capabilities and limitations of the method are evaluated by means of some numerical simulations.
Nonlinear coda wave analysis of hysteretic elastic behavior in strongly scattering media
Ouarabi, M. Ait; Boubenider, F.; Gliozzi, A. S.; Scalerandi, M.
2016-10-01
Strongly scattering elastic media, such as consolidated granular materials, respond to ultrasonic pulse excitations with a long response signal with peculiar properties. The portion of the signal at late times, termed coda, is due to multiple scattering. It contains information about the elastic properties of the material, and it has been proven to be very sensitive to small variations in the modulus. Here we propose a technique based on a nonlinear analysis of the coda of a signal, which might be applied to quantify the nonlinear elastic response in consolidated granular media exhibiting a hysteretic elastic behavior. The method proposed allows for an intrinsic definition of the reference signal which is normally needed for applying coda-based methods.
Ellison, Donald C; Bykov, Andrei M
2015-01-01
We include a general form for the scattering mean free path in a nonlinear Monte Carlo model of relativistic shock formation and Fermi acceleration. Particle-in-cell (PIC) simulations, as well as analytic work, suggest that relativistic shocks tend to produce short-scale, self-generated magnetic turbulence that leads to a scattering mean free path (mfp) with a stronger momentum dependence than the mfp ~ p dependence for Bohm diffusion. In unmagnetized shocks, this turbulence is strong enough to dominate the background magnetic field so the shock can be treated as parallel regardless of the initial magnetic field orientation, making application to gamma-ray bursts (GRBs), pulsar winds, Type Ibc supernovae, and extra-galactic radio sources more straightforward and realistic. In addition to changing the scale of the shock precursor, we show that, when nonlinear effects from efficient Fermi acceleration are taken into account, the momentum dependence of the mfp has an important influence on the efficiency of cosm...
Nonlinear Time Series Analysis of White Dwarf Light Curves
Jevtic, N.; Zelechoski, S.; Feldman, H.; Peterson, C.; Schweitzer, J.
2001-12-01
We use nonlinear time series analysis methods to examine the light intensity curves of white dwarf PG1351+489 obtained by the Whole Earth Telescope (WET). Though these methods were originally introduced to study chaotic systems, when a clear signature of determinism is found for the process generating an observable and it couples the active degrees of freedom of the system, then the notion of phase space provides a framework for exploring the system dynamics of nonlinear systems in general. With a pronounced single frequency, its harmonics and other frequencies of lower amplitude on a broadband background, the PG1351 light curve lends itself to the use of time delay coordinates. Our phase space reconstruction yields a triangular, toroidal three-dimensional shape. This differs from earlier results of a circular toroidal representation. We find a morphological similarity to a magnetic dynamo model developed for fast rotators that yields a union of both results: the circular phase space structure for the ascending portion of the cycle, and the triangular structure for the declining portion. The rise and fall of the dynamo cycle yield both different phase space representations and different correlation dimensions. Since PG1351 is known to have no significant fields, these results may stimulate the observation of light curves of known magnetic white dwarfs for comparison. Using other data obtained by the WET, we compare the phase space reconstruction of DB white dwarf PG1351 with that of GD 358 which has a more complex power spectrum. We also compare these results with those for PG1159. There is some general similarity between the results of the phase space reconstruction for the DB white dwarfs. As expected, the difference between the results for the DB white dwarfs and PG1159 is great.
Zhang, Lin
2012-01-01
High-gain resonant nonlinear Raman scattering on trapped cold atoms within a high-fineness ring optical cavity is simply explained under a nonlinear opto-mechanical mechanism, and a proposal using it to detect frequency of micro-trap on atom chip is presented. The enhancement of scattering spectrum is due to coherent Raman conversion between two different cavity modes mediated by collective vibrations of atoms through nonlinear opto-mechanical couplings. The physical conditions of this technique are roughly estimated on Rubidium atoms, and a simple quantum analysis as well as a multi-body semiclassical simulation on this nonlinear Raman process is conducted.
Light collection from scattering media in a silicon photonics integrated circuit
2011-01-01
We present a silicon photonics integrated circuit to efficiently couple scattered light into a single mode waveguide. By modulating the phase of N light-capturing elements, the collection efficiency can be increased by a factor N.
Focusing light through scattering media by full-polarization digital optical phase conjugation.
Shen, Yuecheng; Liu, Yan; Ma, Cheng; Wang, Lihong V
2016-03-15
Digital optical phase conjugation (DOPC) is an emerging technique for focusing light through or within scattering media such as biological tissue. Since DOPC systems are based on time reversal, they benefit from collecting as much information about the scattered light as possible. However, existing DOPC techniques record and subsequently phase-conjugate the scattered light in only a single-polarization state, limited by the operating principle of spatial light modulators. Here, we develop the first, to the best of our knowledge, full-polarization DOPC system that records and phase-conjugates scattered light along two orthogonal polarizations. When focusing light through thick scattering media, such as 2 mm and 4 mm-thick chicken breast tissue, our full-polarization DOPC system on average doubles the focal peak-to-background ratio achieved by single-polarization DOPC systems and improves the phase-conjugation fidelity.
Spatiotemporal focusing in opaque scattering media by wave front shaping with nonlinear feedback.
Aulbach, Jochen; Gjonaj, Bergin; Johnson, Patrick; Lagendijk, Ad
2012-12-31
We experimentally demonstrate spatiotemporal focusing of light on single nanocrystals embedded inside a strongly scattering medium. Our approach is based on spatial wave front shaping of short pulses, using second harmonic generation inside the target nanocrystals as the feedback signal. We successfully develop a model both for the achieved pulse duration as well as the observed enhancement of the feedback signal. The approach enables exciting opportunities for studies of light propagation in the presence of strong scattering as well as for applications in imaging, micro- and nanomanipulation, coherent control and spectroscopy in complex media.
Study of the nanobubble phase of aqueous NaCl solutions by dynamic light scattering
Energy Technology Data Exchange (ETDEWEB)
Bunkin, N F; Shkirin, A V [A M Prokhorov General Physics Institute, Russian Academy of Sciences, Moscow (Russian Federation); Burkhanov, I S; Chaikov, L L [P N Lebedev Physics Institute, Russian Academy of Sciences, Moscow (Russian Federation); Lomkova, A K [N.E. Bauman Moscow State Technical University, Moscow (Russian Federation)
2014-11-30
Aqueous NaCl solutions with different concentrations have been investigated by dynamic scattering of laser radiation. It is experimentally shown that these solutions contain scattering particles with a wide size distribution in a range of ∼10 – 100 nm. The experimental results indirectly confirm the existence of quasi-stable gas nanobubbles in the bulk of aqueous ionic solutions. (light scattering)
Kawauchi, Satoko; Sato, Shunichi; Ooigawa, Hidetoshi; Nawashiro, Hiroshi; Ishihara, Miya; Kikuchi, Makoto
2009-08-14
Measurement of intrinsic optical signals (IOSs) is an attractive technique for monitoring tissue viability in brains since it enables noninvasive, real-time monitoring of morphological characteristics as well as physiological and biochemical characteristics of tissue. We previously showed that light scattering signals reflecting cellular morphological characteristics were closely related to the IOSs associated with the redox states of cytochrome c oxidase in the mitochondrial respiratory chain. In the present study, we examined the relationship between light scattering and energy metabolism. Light scattering signals were transcranially measured in rat brains after oxygen and glucose deprivation, and the results were compared with concentrations of cerebral adenosine triphosphate (ATP) measured by luciferin-luciferase bioluminescence assay. Electrophysiological signal was also recorded simultaneously. After starting saline infusion, EEG activity ceased at 108+/-17s, even after which both the light scattering signal and ATP concentration remained at initial levels. However, light scattering started to change in three phases at 236+/-15s and then cerebral ATP concentration started to decrease at about 260s. ATP concentration significantly decreased during the triphasic scattering change, indicating that the start of scattering change preceded the loss of cerebral ATP. The mean time difference between the start of triphasic scattering change and the onset of ATP loss was about 24s in the present model. DC potential measurement showed that the triphasic scattering change was associated with anoxic depolarization. These findings suggest that light scattering signal can be used as an indicator of loss of tissue viability in brains.
Generation of Attosecond X-Ray Pulse through Coherent Relativistic Nonlinear Thomson Scattering
Lee, K; Jeong, Y U; Lee, B C; Park, S H
2005-01-01
In contrast to some recent experimental results, which state that the Nonlinear Thomson Scattered (NTS) radiation is incoherent, a coherent condition under which the scattered radiation of an incident laser pulse by a bunch of electrons can be coherently superposed has been investigated. The Coherent Relativistic Nonlinear Thomson Scattered (C-RNTS) radiation makes it possible utilizing the ultra-short pulse nature of NTS radiation with a bunch of electrons, such as plasma or electron beams. A numerical simulation shows that a 25 attosecond X-ray pulse can be generated by irradiating an ultra-intense laser pulse of 4x10(19) W/cm2 on an ultra-thin solid target of 50 nm thickness, which is commercially available. The coherent condition can be easily extended to an electron beam from accelerators. Different from the solid target, much narrower electron beam is required for the generation of an attosecond pulse. Instead, this condition could be applied for the generation of intense Compton scattered X-rays with a...
Institute of Scientific and Technical Information of China (English)
ZHAO XiaoHui; HUANG ChengZhi
2007-01-01
In acid buffer solution, proteins with positive charge can react with anion surfactant and result in a great enhancement of synchronous light scattering (SLS) signals. In this contribution, the correlative experiment was made to compare the interaction of human serum albumin (HAS) and immunoglobulin G (IgG) with sodium dodecyl sulfonate (SDS). Based on the measurements of the polarization light scattering signals, a new method of scattering polarization was constituted to distinguish these two interaction systems with molecular weight difference (HAS 66 kDa; IgG 150 kDa). The results were consistent with the data measured by dynamic light scattering (DLS) technique.
Li, Xu; Chen, Zhigang; Gong, Jianmin; Taflove, Allen; Backman, Vadim
2004-06-01
Understanding light scattering by nonspherical particles is crucial in modeling the transport of light in realistic structures such as biological tissues. We report the application of novel analytical approaches based on modified Wentzel-Kramers-Brillouin and equiphase-sphere methods that facilitate accurate characterization of light scattering by a wide range of irregularly shaped dielectric particles. We also demonstrate that these approaches have the potential to address the inverse-scattering problem by means of a spectral analysis of the total scattering cross section of arbitrarily shaped particles.
Spatio-Temporal Imaging of Light Transport in Highly Scattering Media under White Light Illumination
Badon, Amaury; Lerosey, Geoffroy; Boccara, Albert C; Fink, Mathias; Aubry, Alexandre
2016-01-01
Imaging the propagation of light in time and space is crucial in optics, notably for the study of complex media. We here demonstrate the passive measurement of time-dependent Green's functions between every point at the surface of a strongly scattering medium by means of low coherence interferometry. The experimental access to this Green's matrix is essential since it contains all the information about the complex trajectories of light within the medium. In particular, the spatio-temporal spreading of the diffusive halo can be locally investigated in the vicinity of each point then acting as a virtual source. On the one hand, this approach allows a quantitative imaging of the diffusion constant in the scattering medium with a spatial resolution of the order of a few transport mean free paths. On the other hand, our approach is able to reveal and quantify the anisotropy of light diffusion, which can be of great interest for optical characterization purposes. This study opens important perspectives both in opti...
Optical evaluation of Fricke xylenol orange gel by light scattered at 90 degrees
Energy Technology Data Exchange (ETDEWEB)
Svoboda, J; Alwan, R; Guermeur, F; Makovicka, L; Bailly, Y [IRMA/ENISYS/FEMTO-ST UMR 6174 CNRS, Universite de Franche-Comte, Pole Universitaire, BP 71427, 25211 Montbeliard Cedex (France); Spevacek, V; Cechak, T [Department of Dosimetry and Application of Ionizing Radiation, FNSPE, Czech Technical University in Prague, Brehova 7, Praha 1, 115 19 (Czech Republic); Martin, E [Department of Radiotherapy, CH Belfort-Montbeliard, 25209 Montbeliard (France)], E-mail: svobojir@kmlinux.fjfi.cvut.cz
2009-05-01
This communication presents optical method for evaluation of Fricke xylenol gel (FXG) using light scattered at 90 degrees to initial direction. Although Fricke gel is predominantly absorbing, gelatine matrix scatters enough light which could be collected and related to dose delivered to gel. Initials experiments were oriented to determination applicability of this approach.
Bruining, J.; Fijnaut, H.M.
We have obtained a rotational diffusion coefficient of the 70S ribosome isolated from Escherichia-coli (MRE-600), from the depolarized light scattering spectrum measured by photon correlation spectroscopy. The intensity correlation function of depolarized scattered light contains contributions due
Bruining, J.; Fijnaut, H.M.
1975-01-01
We have obtained a rotational diffusion coefficient of the 70S ribosome isolated from Escherichia-coli (MRE-600), from the depolarized light scattering spectrum measured by photon correlation spectroscopy. The intensity correlation function of depolarized scattered light contains contributions due t
Measurements of strong correlations in the transport of light through strongly scattering materials
Akbulut, D.
2013-01-01
In this thesis, we study light transport through multiple scattering random photonic materials. Light incident on such materials undergoes many scattering events before exiting the material. The relation between the incident and the transmitted fields is determined by the optical transmission matrix
Measurements of strong correlations in the transport of light through strongly scattering materials
Akbulut, D.
2013-01-01
In this thesis, we study light transport through multiple scattering random photonic materials. Light incident on such materials undergoes many scattering events before exiting the material. The relation between the incident and the transmitted fields is determined by the optical transmission matrix
Light-scattering polarization measurements as a new parameter in flow cytometry
Grooth, de B.G.; Terstappen, L.W.M.M.; Puppels, G.J.; Greve, J.
1987-01-01
Polarization measurement of orthogonal light scattering is introduced as a new optical parameter in flow cytometry. In the experimental setup, the electrical field of the incident laser beam is polarized in the direction of the sample flow. The intensity of the orthogonal light scattering polarized
DEFF Research Database (Denmark)
Pilny, Lukas; Bissacco, Giuliano; De Chiffre, Leonardo
The effect of angular orientation of a scattered light sensor with respect to main curvature and surface lay on roughness measurements is evaluated. A commercial scattered light sensor OS 500-32 from Optosurf GmbH was used. The investigation was performed on polished cylindrical surfaces with cro...
Theory of nonlinear phononics for coherent light control of solids
Subedi, Alaska; Cavalleri, Andrea; Georges, Antoine
2014-06-01
We present a microscopic theory for ultrafast control of solids with high-intensity terahertz frequency optical pulses. When resonant with selected infrared-active vibrations, these pulses transiently modify the crystal structure and lead to new collective electronic properties. The theory predicts the dynamical path taken by the crystal lattice using first-principles calculations of the energy surface and classical equations of motion, as well as symmetry considerations. Two classes of dynamics are identified. In the perturbative regime, displacements along the normal mode coordinate of symmetry-preserving Raman active modes can be achieved by cubic anharmonicities. This explains the light-induced insulator-to-metal transition reported experimentally in manganites. We predict a regime in which ultrafast instabilities that break crystal symmetry can be induced. This nonperturbative effect involves a quartic anharmonic coupling and occurs above a critical threshold, below which the nonlinear dynamics of the driven mode displays softening and dynamical stabilization.
Observation of nonlinear resonances in the advanced light source
Robin, D.; Collins, H.; Decking, W.; Portmann, G.; Schachinger, L.; Zholents, A.
1995-09-01
Observations of nonlinear resonances in the Advanced Light Source have been made by scanning betatron tunes and observing count rates in a beam-loss radiation monitor placed down stream of a beam scraper. We have found that it is possible to see structural resonances which are unallowed as well as those which are allowed by the ring's natural 12-fold symmetry. By systematically breaking the amount of symmetry we see that the widths of the unallowed resonances grow while the widths of the allowed resonances do not. In this paper we briefly discuss the importance of symmetry and its effect on resonances in the design of the ALS. Next we describe our experimental setup and discuss the performance of the beam loss monitor which we used to view the resonances. We then present scans of the tune space where one can see the presence of the structural resonances and their evolution when the lattice symmetry is systematically broken.
Characterization of dental composite curing kinetics using dynamic light scattering
Wells-Gray, Elaine M.; Kirkpatrick, Sean J.; Sakaguchi, Ron L.
2009-02-01
Polymer resin composites are a class of widely used restorative dental materials that undergo a complex polymerization curing process that has been the subject of substantial research. This study uses speckle correlation methods based on dynamic light scattering as a tool to monitor the rate and extent of dental composite polymerization during and after photo-curing. Thin disc-shaped samples (composite consisting of 50:50 BisGMA/TEGDMA resin, quartz silica filler particles, and camphorquinone as photo-initiator. A 633 nm HeNe laser beam was used to probe the top surface of the sample via a backscattered speckle pattern, while the bottom surface was illuminated with a halogen curing lamp (peak wavelength=470nm) to initiate the polymerization reaction. The speckle patterns were recorded with a CCD camera, and stored as a 'speckle cube' for post processing. Correlation values of the intensity fluctuation were calculated on a pixel-by-pixel basis for pairs of subsequent speckle images and then ensemble averaged. Results show a sharp decrease in correlation at the onset of curing, indicating a large amount of double bond conversion and movement within the composite. Correlation values then quickly increase, eventually reaching a plateau near unity, indicating cessation of molecular rearrangement. The kinetic behavior demonstrated by our correlation curves are in good agreement with curing data found in the literature, and demonstrate the usefulness of this technique for monitoring dental composite curing.
Physiological and pathological clinical conditions and light scattering in brain
Kurata, Tsuyoshi; Iwata, Sachiko; Tsuda, Kennosuke; Kinoshita, Masahiro; Saikusa, Mamoru; Hara, Naoko; Oda, Motoki; Ohmae, Etsuko; Araki, Yuko; Sugioka, Takashi; Takashima, Sachio; Iwata, Osuke
2016-08-01
MRI of preterm infants at term commonly reveals subtle brain lesions such as diffuse white matter injury, which are linked with later cognitive impairments. The timing and mechanism of such injury remains unclear. The reduced scattering coefficient of near-infrared light (μs’) has been shown to correlate linearly with gestational age in neonates. To identify clinical variables associated with brain μs’, 60 preterm and full-term infants were studied within 7 days of birth. Dependence of μs’ obtained from the frontal head on clinical variables was assessed. In the univariate analysis, smaller μs’ was associated with antenatal glucocorticoid, emergency Caesarean section, requirement for mechanical ventilation, smaller gestational age, smaller body sizes, low 1- and 5-minute Apgar scores, higher cord blood pH and PO2, and higher blood HCO3‑ at the time of study. Multivariate analysis revealed that smaller gestational age, requirement for mechanical ventilation, and higher HCO3‑ at the time of study were correlated with smaller μs’. Brain μs’ depended on variables associated with physiological maturation and pathological conditions of the brain. Further longitudinal studies may help identify pathological events and clinical conditions responsible for subtle brain injury and subsequent cognitive impairments following preterm birth.
Light scattering studies of irradiated {kappa}- and {iota}-carrageenan
Energy Technology Data Exchange (ETDEWEB)
Abad, L.V. [Neutron Science Laboratory, Institute for Solid State Physics, University of Tokyo, 106-1 Shirakata, Tokai, Ibaraki 319-1106 (Japan) and Philippine Nuclear Research Institute, Commonwealth Ave., Diliman, Quezon City (Philippines)]. E-mail: lvabad@pnri.dost.gov.ph; Nasimova, I.R. [Neutron Science Laboratory, Institute for Solid State Physics, University of Tokyo, 106-1 Shirakata, Tokai, Ibaraki 319-1106 (Japan); Physics Department, Moscow State University, Moscow 119992 (Russian Federation); Aranilla, C.T. [Philippine Nuclear Research Institute, Commonwealth Ave., Diliman, Quezon City (Philippines); Shibayama, M. [Neutron Science Laboratory, Institute for Solid State Physics, University of Tokyo, 106-1 Shirakata, Tokai, Ibaraki 319-1106 (Japan)]. E-mail: sibayama@issp.u-tokyo.ac.jp
2005-05-01
The relationships between the molecular weight (Mw) and the characteristic decay time distribution function G({gamma}) of irradiated kappa ({kappa}-) and iota ({iota}-) carrageenan were studied by static and dynamic light scattering (DLS). Mw and the characteristic decay time ({gamma}{sup -1}) are both steep decreasing exponential function with radiation dose. The dynamic behavior of irradiated {iota}-carrageenan was compared to irradiated {kappa}-carrageenan by DLS. The intensity correlation function of both carrageenans shifted towards shorter relaxation times with increasing radiation dose. Irradiated {iota}-carrageenan like {kappa}-carrageenan exhibits power law behavior at 0-50 kGy (at 0.05-0.1M KCl) indicating similar gelation behaviors. The temperature at which transition from coil to helix takes place (conformational transition temperature) decreases with increasing irradiation dose. A new faster relaxation mode appears at around 0.1-1 ms for both carrageenans between 100 and 150 kGy. Maximum peak height for this mode is at 100 kGy which corresponds to the optimum biological activity of {kappa}- and {iota}-carrageenan.
Scattering of electromagnetic light waves from a deterministic anisotropic medium
Li, Jia; Chang, Liping; Wu, Pinghui
2015-11-01
Based on the weak scattering theory of electromagnetic waves, analytical expressions are derived for the spectral densities and degrees of polarization of an electromagnetic plane wave scattered from a deterministic anisotropic medium. It is shown that the normalized spectral densities of scattered field is highly dependent of changes of the scattering angle and degrees of polarization of incident plane waves. The degrees of polarization of scattered field are also subjective to variations of these parameters. In addition, the anisotropic effective radii of the dielectric susceptibility can lead essential influences on both spectral densities and degrees of polarization of scattered field. They are highly dependent of the effective radii of the medium. The obtained results may be applicable to determine anisotropic parameters of medium by quantitatively measuring statistics of a far-zone scattered field.
Energy Technology Data Exchange (ETDEWEB)
Maxein, Karl Dominik
2009-12-15
Lithium niobate (LiNbO{sub 3}) is a widely employed material in nonlinear optics and photonics. Its usage is hampered by the photorefractive effect, which can destroy beam profiles and phase matching conditions. Existing methods to suppress photorefraction fail for the interesting regime of very high intensities and short pulses. Therefore, the photorefractive effect is investigated using femtosecond laser pulses: By utilizing so-called 2K holography, the occupation of energetically shallow traps is observed to occur in less than 100 fs after a two-photon excitation. Writing of photorefractive gratings into oxidized iron-doped LiNbO{sub 3} is much faster with pulses than with cw light. This is explained by the sensitization of the crystal due to charge trapping in photorefractive centers after nonlinear excitations. Finally, light-induced scattering of pulse light is suppressed compared to the scattering of cw light due to the small coherence length of pulses. (orig.)
Directory of Open Access Journals (Sweden)
Luisa A Marcelino
Full Text Available Calcium carbonate skeletons of scleractinian corals amplify light availability to their algal symbionts by diffuse scattering, optimizing photosynthetic energy acquisition. However, the mechanism of scattering and its role in coral evolution and dissolution of algal symbioses during "bleaching" events are largely unknown. Here we show that differences in skeletal fractal architecture at nano/micro-lengthscales within 96 coral taxa result in an 8-fold variation in light-scattering and considerably alter the algal light environment. We identified a continuum of properties that fall between two extremes: (1 corals with low skeletal fractality that are efficient at transporting and redistributing light throughout the colony with low scatter but are at higher risk of bleaching and (2 corals with high skeletal fractality that are inefficient at transporting and redistributing light with high scatter and are at lower risk of bleaching. While levels of excess light derived from the coral skeleton is similar in both groups, the low-scatter corals have a higher rate of light-amplification increase when symbiont concentration is reduced during bleaching, thus creating a positive feedback-loop between symbiont concentration and light-amplification that exposes the remaining symbionts to increasingly higher light intensities. By placing our findings in an evolutionary framework, in conjunction with a novel empirical index of coral bleaching susceptibility, we find significant correlations between bleaching susceptibility and light-scattering despite rich homoplasy in both characters; suggesting that the cost of enhancing light-amplification to the algae is revealed in decreased resilience of the partnership to stress.
Recursion relations and scattering amplitudes in the light-front formalism
Cruz-Santiago, Christian A
2013-01-01
The fragmentation functions and scattering amplitudes are investigated in the framework of light-front perturbation theory. It is demonstrated that, the factorization property of the fragmentation functions implies the recursion relations for the off-shell scattering amplitudes which are light-front analogs of the Berends-Giele relations. These recursion relations on the light-front can be solved exactly by induction and it is shown that the expressions for the off-shell light-front amplitudes are represented as a linear combinations of the on-shell amplitudes. By putting external particles on-shell we recover the scattering amplitudes previously derived in the literature.
Towards a data-driven analysis of hadronic light-by-light scattering
Colangelo, Gilberto; Kubis, Bastian; Procura, Massimiliano; Stoffer, Peter
2014-01-01
The hadronic light-by-light contribution to the anomalous magnetic moment of the muon was recently analyzed in the framework of dispersion theory, providing a systematic formalism where all input quantities are expressed in terms of on-shell form factors and scattering amplitudes that are in principle accessible in experiment. We briefly review the main ideas behind this framework and discuss the various experimental ingredients needed for the evaluation of one- and two-pion intermediate states. In particular, we identify processes that in the absence of data for doubly-virtual pion-photon interactions can help constrain parameters in the dispersive reconstruction of the relevant input quantities, the pion transition form factor and the helicity partial waves for $\\gamma^*\\gamma^*\\to\\pi\\pi$.
Light Conversion and Scattering in UV Protective Textiles
Directory of Open Access Journals (Sweden)
Grancarić Ana Marija
2014-12-01
Full Text Available The primary cause of skin cancer is believed to be a long exposure to solar ultraviolet radiation (UV-R crossed with the amount of skin pigmentation in the population. It is believed that in childhood and adolescence 80% of UV-R gets absorbed, whilst in the remaining 20% gets absorbed later in the lifetime. This suggests that proper and early photoprotection may reduce the risk of subsequent occurrence of skin cancer. Textile and clothing are the most suitable interface between environment and human body. It can show UV protection, but in most cases it does not provide full sun screening properties. UV protection ability highly depends on large number of factors such as type of fibre, fabric surface and construction, type and concentration of dyestuff, fluorescent whitening agent (FWA, UV-B protective agents, as well as nanoparticles, if applied. Based on electronically excited state by energy of UV-R (usually 340-370 nm, the molecules of FWAs show the phenomenon of fluorescence giving to white textiles high whiteness of outstanding brightness by reemitting the energy at the blue region (typically 420-470 nm of the spectrum. By absorbing UV-A radiation, optical brightened fabrics transform this radiation into blue fluorescence, which leads to better UV protection. Natural zeolites are rock-forming, microporous silicate minerals. Applied as nanoparticles to textile surface, it scatters the UV-R resulting in lower UV-A and UV-B transmission. If applied with other UV absorbing agents, e.g. FWAs, synergistic effect occurs. Silicones are inert, synthetic compounds with a variety of forms and uses. It provides a unique soft touch, is very resistant to washing and improves the property of fabric to protect against UV radiation. Therefore, the UV protective properties of cotton fabric achieved by light conversion and scattering was researched in this paper. For that purpose, the stilbene-derived FWAs were applied on cotton fabric in wide concentration
Ultraslow-light effects in symmetric and asymmetric waveguide structures with moon-like scatterers
Wan, Yong; Ge, Xiao-Hui; Xu, Sheng; Guo, Yue; Yuan, Feng
2017-02-01
Ultraslow-light effects in two-dimensional hexagonal-lattice coupled waveguide with moon-like scatterers were theoretically studied using the plane-wave expansion method. For symmetric structures, simulations showed that slow light with high group index can be achieved by shifting the scatterers and adjusting the radius of moon-like scatterers. The maximum group index was over 8:0 × 104. For asymmetric structures, simulations showed that slow light with flat band and high group index can be obtained by shifting the scatterers, adjusting the radius of moon-like scatterers, and rotating the scatterers. The maximum group index was over 5:7 × 105 with a "saddle-like" relationship between the frequency and group index.
Werner, Liliana; Morris, Caleb; Liu, Erica; Stallings, Shannon; Floyd, Anne; Ollerton, Andrew; Leishman, Lisa; Bodnar, Zachary
2014-01-01
To assess the potential effect of surface light scattering on light transmittance of 1-piece hydrophobic acrylic intraocular lenses (IOLs) with or without a blue-light filter. John A. Moran Eye Center, University of Utah, Salt Lake City, Utah, USA. Experimental study. Intraocular lenses were obtained from human cadavers (49 IOLs total; 36 with blue-light filter) and from finished-goods inventory (controls). The IOLs were removed from cadaver eyes and the power and model matched to unused controls. After surface proteins were removed, the IOLs were hydrated for 24 hours at room temperature. Surface light scattering was measured with a Scheimpflug camera (EAS-1000 Anterior Segment Analysis System). Light transmittance was measured with a Lambda 35 UV/Vis spectrophotometer (single-beam configuration; RSA-PE-20 integrating sphere). Hydrated scatter values ranged from 4.8 to 202.5 computer-compatible tape (CCT) units for explanted IOLs with blue-light filter and 1.5 to 11.8 CCT units for controls; values ranged from 6.0 to 137.5 CCT units for explanted IOLs without a blue-light filter and 3.5 to 9.6 CCT units for controls. In both groups, there was a tendency toward increasing scatter values with increasing postoperative time. No differences in light transmittance were observed between explanted IOLs and controls in both groups (IOLs with blue-light filter: P=.407; IOL with no blue-light filter: P=.487; both paired t test). Although surface light scattering of explanted IOLs was significantly higher than that of controls and appeared to increase with time, no effect was observed on light transmittance of 1-piece hydrophobic acrylic IOLs with or without a blue-light filter. Copyright © 2013 ASCRS and ESCRS. Published by Elsevier Inc. All rights reserved.
Ellison, Donald C.; Warren, Donald C.; Bykov, Andrei M.
2016-03-01
We include a general form for the scattering mean free path, λmfp(p), in a nonlinear Monte Carlo model of relativistic shock formation and Fermi acceleration. Particle-in-cell simulations, as well as analytic work, suggest that relativistic shocks tend to produce short-scale, self-generated magnetic turbulence that leads to a scattering mean free path with a stronger momentum dependence than the λmfp ∝ p dependence for Bohm diffusion. In unmagnetized shocks, this turbulence is strong enough to dominate the background magnetic field so the shock can be treated as parallel regardless of the initial magnetic field orientation, making application to γ-ray bursts, pulsar winds, type Ibc supernovae, and extragalactic radio sources more straightforward and realistic. In addition to changing the scale of the shock precursor, we show that, when nonlinear effects from efficient Fermi acceleration are taken into account, the momentum dependence of λmfp(p) has an important influence on the efficiency of cosmic ray production as well as the accelerated particle spectral shape. These effects are absent in non-relativistic shocks and do not appear in relativistic shock models unless nonlinear effects are self-consistently described. We show, for limited examples, how the changes in Fermi acceleration translate to changes in the intensity and spectral shape of γ-ray emission from proton-proton interactions and pion-decay radiation.
Jacques, Steven L.; Roussel, Stéphane; Samatham, Ravikant
2016-01-01
Abstract. This report describes how optical images acquired using linearly polarized light can specify the anisotropy of scattering (g) and the ratio of reduced scattering [μs′=μs(1−g)] to absorption (μa), i.e., N′=μs′/μa. A camera acquired copolarized (HH) and crosspolarized (HV) reflectance images of a tissue (skin), which yielded images based on the intensity (I=HH+HV) and difference (Q=HH−HV) of reflectance images. Monte Carlo simulations generated an analysis grid (or lookup table), which mapped Q and I into a grid of g versus N′, i.e., g(Q,I) and N′(Q,I). The anisotropy g is interesting because it is sensitive to the submicrometer structure of biological tissues. Hence, polarized light imaging can monitor shifts in the submicrometer (50 to 1000 nm) structure of tissues. The Q values for forearm skin on two subjects (one Caucasian, one pigmented) were in the range of 0.046±0.007 (24), which is the mean±SD for 24 measurements on 8 skin sites×3 visible wavelengths, 470, 524, and 625 nm, which indicated g values of 0.67±0.07 (24). PMID:27165546
Doc, Jean-Baptiste; Conoir, Jean-Marc; Marchiano, Régis; Fuster, Daniel
2016-04-01
The weakly nonlinear propagation of acoustic waves in monodisperse bubbly liquids is investigated numerically. A hydrodynamic model based on the averaged two-phase fluid equations is coupled with the Rayleigh-Plesset equation to model the dynamics of bubbles at the local scale. The present model is validated in the linear regime by comparing with the Foldy approximation. The analysis of the pressure signals in the linear regime highlights two resonance frequencies: the Minnaert frequency and a multiple scattering resonance that strongly depends on the bubble concentration. For weakly nonlinear regimes, the generation of higher harmonics is observed only for the Minnaert frequency. Linear combinations between the Minnaert harmonics and the multiple scattering resonance are also observed. However, the most significant effect observed is the appearance of softening-hardening effects that share some similarities with those observed for sandstones or cracked materials. These effects are related to the multiple scattering resonance. Downward or upward resonance frequency shifts can be observed depending on the characteristic of the incident wave when increasing the excitation amplitude. It is shown that the frequency shift can be explained assuming that the acoustic wave velocity depends on a law different from those usually encountered for sandstones or cracked materials.
Adkins, Gregory S; Salinger, M D; Wang, Ruihan; Fell, Richard N
2014-01-01
Recent and ongoing experimental work on the positronium spectrum motivates new efforts to calculate positronium energy levels at the level of three loop corrections. We have obtained results for one set of such corrections involving light-by-light scattering of the photons produced in a two-photon virtual annihilation process. Our result is an energy shift $1.58377(8) m \\alpha^7/\\pi^3$ for the n=1 singlet state, correcting the ground state hyperfine splitting by -6.95 kHz. We also obtained a new and more precise result for the light-by-light scattering correction to the real decay of parapositronium into two photons.
Polarization control of multiply-scattered light through random media by wavefront shaping
Guan, Yefeng; Small, Eran; Zhou, Jianying; Silberberg, Yaron
2015-01-01
We show that the polarization state of coherent light propagating through an optically thick multiple-scattering medium, can be controlled by wavefront shaping, i.e. by controlling only the spatial phase of the incoming field with a spatial light modulator. Any polarization state of light at any spatial position behind the scattering medium can be attained with this technique. Thus, transforming the random medium to an arbitrary optical polarization component becomes possible.
Ceolato, Romain; Riviere, Nicolas
2016-07-01
Spectral polarimetric light-scattering by particulate media has recently attracted growing interests for various applications due to the production of directional broadband light sources. Here the spectral polarimetric light-scattering signatures of particulate media are simulated using a numerical model based on the spectral Vector Radiative Transfer Equation (VRTE). A microphysical analysis is conducted to understand the dependence of the light-scattering signatures upon the microphysical parameters of particles. We reveal that depolarization from multiple scattering results in remarkable spectral and directional features, which are simulated by our model over a wide spectral range from visible to near-infrared. We propose to use these features to improve the inversion of the scattering problem in the fields of remote sensing, astrophysics, material science, or biomedical.
Enhancing light transmission through a random medium with inhomogeneous scattering and loss
Sarma, Raktim; Cao, Hui
2016-01-01
We enhanced the total transmission of light through a disordered waveguide with spatially inhomogeneous scattering and loss by shaping the incident wavefront of a laser beam. Using an on-chip tapered lead, we were able to access all input modes in the waveguide with a spatial light modulator. The adaptive wavefront shaping resulted in selective coupling of input light to high transmission channels, which bypassed the regions of higher scattering and loss in the waveguide. The spatial inhomogeneity of scattering and loss led to redirecting of energy flux to optical paths with less scattering and loss to maximize total energy transported through the system. This work demonstrated the power of wavefront shaping in coherent control of light transport in inhomogeneous scattering media, which are common in real applications.
Eremin, Yuri; Wriedt, Thomas
2014-12-01
The Discrete Sources Method (DSM) has been modified to analyze polarized light scattering by an axial symmetric penetrable nanoparticle partially embedded into a substrate. The new numerical scheme of the DSM enables to consider scattering from such substrate defects as flat particles, mounds, pits and voids. A detailed description of the numerical scheme is provided. The developed computer model has been employed to investigate scattering from a shallow particle and pit. Simulation results corresponding to the Differential Scattering Cross-Section and the integral response for P/S polarized light are presented.
UV Nano-Lights: Nonlinear Quantum Dot-Plasmon Coupling
2014-08-01
method is also applicable to bare nanoparticles in polar solvents. 15. SUBJECT TERMS Quantum Dots, Nonlinear Optical Materials , Energy...TERMS Quantum Dots, Nonlinear Optical Materials , Energy Conservation, Up-conversion 16. SECURITY CLASSIFICATION OF: 17. LIMITATION OF ABSTRACT
Shiraya, Tomoyasu; Kato, Satoshi; Minami, Keiichiro; Miyata, Kazunori
2017-02-01
The aim of this study was to experimentally examine the changes in the transmittances of photocoagulation lasers when surface light scattering increases in AcrySof intraocular lenses (IOLs). SA60AT IOLs (Alcon) were acceleratingly aging for 0, 3, 5, and 10 years to simulate surface light scattering, and the surface light-scattering intensities of both IOL surfaces were measured using a Scheimpflug photographer. The powers of laser beams that passed from a laser photocoagulator through the aged IOLs were measured at 532, 577, and 647 nm. Changes in the laser power and transmittance with the years of aging and the intensities of surface light scattering were examined. Although the intensity of surface light scattering increased with the years of aging, the laser power did not change with the years of aging (P > 0.30, Kruskal-Wallis test). There were no significant changes in the laser transmittance with the years of aging or the laser wavelength (P > 0.30 and 0.57, respectively). The intensity of surface light scattering revealed no significant association with the laser transmittance at any wavelength (P > 0.37, liner regression). The increases in the surface light scattering of the AcrySof IOLs would not influence retinal photocoagulation treatments for up to 10 years after implantation.
Information-theoretic analysis of a stimulated-Brillouin-scattering-based slow-light system.
Lee, Myungjun; Zhu, Yunhui; Gauthier, Daniel J; Gehm, Michael E; Neifeld, Mark A
2011-11-10
We use an information-theoretic method developed by Neifeld and Lee [J. Opt. Soc. Am. A 25, C31 (2008)] to analyze the performance of a slow-light system. Slow-light is realized in this system via stimulated Brillouin scattering in a 2 km-long, room-temperature, highly nonlinear fiber pumped by a laser whose spectrum is tailored and broadened to 5 GHz. We compute the information throughput (IT), which quantifies the fraction of information transferred from the source to the receiver and the information delay (ID), which quantifies the delay of a data stream at which the information transfer is largest, for a range of experimental parameters. We also measure the eye-opening (EO) and signal-to-noise ratio (SNR) of the transmitted data stream and find that they scale in a similar fashion to the information-theoretic method. Our experimental findings are compared to a model of the slow-light system that accounts for all pertinent noise sources in the system as well as data-pulse distortion due to the filtering effect of the SBS process. The agreement between our observations and the predictions of our model is very good. Furthermore, we compare measurements of the IT for an optimal flattop gain profile and for a Gaussian-shaped gain profile. For a given pump-beam power, we find that the optimal profile gives a 36% larger ID and somewhat higher IT compared to the Gaussian profile. Specifically, the optimal (Gaussian) profile produces a fractional slow-light ID of 0.94 (0.69) and an IT of 0.86 (0.86) at a pump-beam power of 450 mW and a data rate of 2.5 Gbps. Thus, the optimal profile better utilizes the available pump-beam power, which is often a valuable resource in a system design.
Muñoz, O.; Hovenier, J.W.
2011-01-01
In this paper we present an overview of light scattering experiments devoted to measure one or more elements of the scattering matrix as functions of the scattering angle of ensembles of randomly oriented small irregular particles in air. A summary of the most important findings in light scattering
DEFF Research Database (Denmark)
Mirzaev, S. Z.; Behrends, R.; Heimburg, Thomas Rainer
2006-01-01
2,6-dimethylpyridine-water, specific heat, dynamic light scattering, shear viscosity Udgivelsesdato: 14 April......2,6-dimethylpyridine-water, specific heat, dynamic light scattering, shear viscosity Udgivelsesdato: 14 April...
Solution of the nonlinear inverse scattering problem by T -matrix completion. II. Simulations
Levinson, Howard W.; Markel, Vadim A.
2016-10-01
This is Part II of the paper series on data-compatible T -matrix completion (DCTMC), which is a method for solving nonlinear inverse problems. Part I of the series [H. W. Levinson and V. A. Markel, Phys. Rev. E 94, 043317 (2016), 10.1103/PhysRevE.94.043317] contains theory and here we present simulations for inverse scattering of scalar waves. The underlying mathematical model is the scalar wave equation and the object function that is reconstructed is the medium susceptibility. The simulations are relevant to ultrasound tomographic imaging and seismic tomography. It is shown that DCTMC is a viable method for solving strongly nonlinear inverse problems with large data sets. It provides not only the overall shape of the object, but the quantitative contrast, which can correspond, for instance, to the variable speed of sound in the imaged medium.
Optical transistor action by nonlinear coupling of stimulated emission and coherent scattering
Andrews, David L.; Bradshaw, David S.
2010-08-01
In the pursuit of improved platforms for computing, communications and internet connectivity, all-optical systems offer excellent prospects for a speed and fidelity of data transmission that will greatly surpass conventional electronics, alongside the anticipated benefits of reduced energy loss. With a diverse range of sources and fiber optical connections already in production, much current effort is being devoted towards forging optical components for signal switching, such as an all-optical transistor. Achievement of the desired characteristics for any practicable device can be expected to depend crucially on the engagement of a strongly nonlinear optical response. The innovative scheme proposed in the present work is based upon a third-order nonlinearity - its effect enhanced by stimulated emission - operating within a system designed to exploit the highly nonlinear response observed at the threshold for laser emission. Here, stimulated emission is strongly driven by coupling to the coherent scattering of a signal input beam whose optical frequency is purposely off-set from resonance. An electrodynamical analysis of the all-optical coupling process shows that the signal beam can significantly modify the kinetics of emission, and so lead to a dramatically enhanced output of resonant radiation. The underlying nonlinear optical mechanism is analyzed, model calculations are performed for realizable three-level laser systems, and the results exhibited graphically. The advantages of implementing this all-optical transistor scheme, compared to several previously envisaged proposals, are then outlined.
Doyuran, Adnan; Joshi, Chandrashekhar; Lim, Jae; Rosenzweig, James E; Tochitsky, Sergei Ya; Travish, Gil; Williams, Oliver
2005-01-01
An Inverse Compton Scattering (ICS) experiment investigating the polarized harmonic production in the nonlinear regime has begun which will utilize the existing terawatt CO2 laser system and 15 MeV photoinjector in the Neptune Laboratory at UCLA. A major motivation for a source of high brightness polarized x-rays is the production of polarized positrons for use in future linear collider experiments. Analytical calculations have been performed to predict the angular and frequency spectrums for various polarizations and different scattering angles. Currently, the experiment is running and we report the set-up and initial results. The advantages and limitations of using a high laser vector potential, ao, in an ICS-based polarized positron source are expected to be revealed with further measurement of the harmonic spectrum and angular characteristics.
Analysis of key properties for optical power limiting and the influence of nonlinear scattering
Koerber, M.; Azarian, A.; Schwarz, B.; Eberle, B.
2014-10-01
In this paper, we propose ways to study the optical limiting behavior of dissolved nanoparticles. We want to present two different approaches. First, we identify the key properties responsible for the critical fluence threshold using a principal component analysis. For metallic nanoparticles, we found that the real part of the complex dielectric function must have a negative value as low as possible, while the imaginary part must be close to zero. Additionally, the solvent should have a low refractive index as well as a low absorption. Furthermore, nonlinear scattering seems to be an important limiting mechanism for nanoparticle limiters. Here, we present a thermal finite element model to predict the temporal evolution of the temperature profile in the nanoparticles and their vicinity. The temperature profile leads to vapor bubbles around the nanoparticles and Mie theory is used to calculate the induced scattering. We demonstrate the functionality of the model by simulating an Au-nanoparticle in an ethanol solution.
Light scattering changes follow evoked potentials from hippocampal Schaeffer collateral stimulation
DEFF Research Database (Denmark)
Rector, D M; Poe, G R; Kristensen, Morten Pilgaard
1997-01-01
-coupled device camera to detect scattered light changes, was lowered to the contralateral dorsal hippocampal surface. Light at 660 +/- 10 (SE) nm illuminated the tissue through optic fibers surrounding the optic probe. An attached bipolar electrode recorded evoked right hippocampal commissural potentials......We assessed relationships of evoked electrical and light scattering changes from cat dorsal hippocampus following Schaeffer collateral stimulation. Under anesthesia, eight stimulating electrodes were placed in the left hippocampal CA field and an optic probe, coupled to a photodiode or a charge...... a complex population synaptic potential that lasted 100-200 ms depending on stimulus intensity and electrode position. Light scattering changes peaked 20 ms after stimuli and occurred simultaneously with population spikes. A long-lasting light scattering component peaked 100-500 ms after the stimulus...
Institute of Scientific and Technical Information of China (English)
TU Juan; GUAN J.F.; MATULA T.J.; Crum L.A.; WEI Rong-jue
2008-01-01
The dynamic behaviour of SonoVue microbubbles a new generation ultrasound contrast agent is investigated in real time with light scattering method.Highly diluted SonoVue microbubbles are injected into a diluted gel made of xanthan gum and water.The responses of individual SonoVue bubbles to driven ultrasound pulses are measured.Both linear and nonlinear bubble oscillations are observed and the results suggest that SonoVue microbubbles can generate strong nonlinear responses.By fitting the experimental data of individual bubble responses with Sarkar's model,the shell coating parameter of the bubbles and dilatational viscosity is estimated to be 7.0 nm·s·Pa.
DEFF Research Database (Denmark)
Andersen, Lasse Mejling; McKinstrie, C. J.; Rottwitt, Karsten
2013-01-01
Recently, we solved the coupled-mode equations for Bragg scattering (BS) in the low- and high-conversion regimes, but without the effects of nonlinear phase modulation (NPM). We now present solutions and Green functions in the low-conversion regime that include NPM. We find that NPM does not change...... are still possible, even when the effects of NPM are included. Finally, the effects of using different input signals are considered, and we conclude that using the natural input modes of the system drastically increases the efficiency. © (2013) COPYRIGHT Society of Photo-Optical Instrumentation Engineers...
Ostrovsky, Lev A; Sutin, Alexander M; Soustova, Irina A; Matveyev, Alexander L; Potapov, Andrey I; Kluzek, Zigmund
2003-02-01
The paper describes nonlinear effects due to a biharmonic acoustic signal scattering from air bubbles in the sea. The results of field experiments in a shallow sea are presented. Two waves radiated at frequencies 30 and 31-37 kHz generated backscattered signals at sum and difference frequencies in a bubble layer. A motorboat propeller was used to generate bubbles with different concentrations at different times, up to the return to the natural subsurface layer. Theoretical consideration is given for these effects. The experimental data are in a reasonably good agreement with theoretical predictions.
Nonlinear kinetic modeling and simulations of Raman scattering in a two-dimensional geometry
Directory of Open Access Journals (Sweden)
Bénisti Didier
2013-11-01
Full Text Available In this paper, we present our nonlinear kinetic modeling of stimulated Raman scattering (SRS by the means of envelope equations, whose coefficients have been derived using a mixture of perturbative and adiabatic calculations. First examples of the numerical resolution of these envelope equations in a two-dimensional homogeneous plasma are given, and the results are compared against those of particle-in-cell (PIC simulations. These preliminary comparisons are encouraging since our envelope code provides threshold intensities consistent with those of PIC simulations while requiring computational resources reduced by 4 to 5 orders of magnitude compared to full-kinetic codes.
Wang, Jiao; Xue, Jinhua; Xiao, Xilin; Xu, Li; Jiang, Min; Peng, Pengcheng; Liao, Lifu
2017-12-05
The coordination reaction of thorium (IV) with a ditopic bidentate ligand to form supramolecular polymer was studied by resonance light scattering (RLS) spectra, second-order scattering (SOS) spectra and frequency-doubling scattering (FDS) spectra, respectively. The ditopic bidentate ligand is isophthalaldehyde-tetrapyrrole (IPTP). It was synthesized through a condensation reaction of isophthalaldehyde with pyrrole. The formation of supramolecular polymer results in remarkable intensity enhancements of the three light scattering signals. The maximum scattering wavelengths of RLS, FDS and SOS were 290, 568 and 340nm, respectively. The reaction was used to establish new light scattering methods for the determination of thorium (IV) by using IPTP as probe. Under optimum conditions, the intensity enhancements of RLS, SOS and FDS were directly proportional to the concentration of thorium (IV) in the ranges of 0.01 to 1.2μgmL(-1), 0.05 to 1.2μgmL(-1) and 0.05 to 1.2μgmL(-1), respectively. The detection limits were 0.003μgmL(-1), 0.012μgmL(-1) and 0.021μgmL(-1), respectively. The methods were suitable for analyzing thorium (IV) in actual samples. The results show acceptable recoveries and precision compared with a reference method. Copyright © 2017 Elsevier B.V. All rights reserved.
Equivalence theorem for the spectral density of light waves on weak scattering.
Wang, Tao; Ji, Xiaoling; Zhao, Daomu
2014-07-01
The Equivalence theorem for the spectral density of light waves on weak scattering is discussed. It is shown that when a spatially coherent plane light wave is scattered from two entirely different media, the far-zone spectral density may have identical distribution provided the low-frequency antidiagonal spatial Fourier components of the correlation function of the media are the same. An example of light waves on scattering from a Gaussian Schell model medium is discussed, and the condition on which two different media may produce identical spectral densities is presented.
ARTICLES: Photoinduced light scattering in cerium-doped barium strontium niobate crystals
Voronov, Valerii V.; Dorosh, I. R.; Kuz'minov, Yu S.; Tkachenko, N. V.
1980-11-01
Photoinduced light scattering was observed in cerium-doped (SrxBa1-x)1-y(Nb2O6)y crystals having the composition x = 0.61, y = 0.4993. It was found that this effect is due to holographic amplification of light scattered by crystal defects. An analysis is made of static and dynamic characteristics of self-amplification of scattered light in the crystals. A theoretical model of the process is constructed assuming that the hologram recording process is of the diffusion type. Theoretical results are compared with the experiment.
Photoinduced light scattering in cerium-doped barium strontium niobate crystals
Voronov, V. V.; Dorosh, I. R.; Kuz'minov, Yu. S.; Tkachenko, N. V.
Photoinduced light scattering was observed in cerium-doped (Srx Ba1-x)1-y(Nb2O6)y crystals having the composition x = 0.61, y = 0.4993. It was found that this effect is due to holographic amplification of light scattered by crystal defects. An analysis is made of static and dynamic characteristics of self-amplification of scattered light in the crystals. A theoretical model of the process is constructed assuming that the hologram recording process is of the diffusion type. Theoretical results are compared with the experiment.
Ribosome formation from subunits studied by stopped-flow and Rayleigh light scattering.
Antoun, Ayman; Pavlov, Michael Y.; Tenson, Tanel; Ehrenberg M, M åNs
2004-01-01
Light scattering and standard stopped-flow techniques were used to monitor rapid association of ribosomal subunits during initiation of eubacterial protein synthesis. The effects of the initiation factors IF1, IF2, IF3 and buffer conditions on subunit association were studied along with the role of GTP in this process. The part of light scattering theory that is essential for kinetic measurements is high-lighted in the main text and a more general treatment of Rayleigh scattering from macromolecules is given in an appendix.
Ribosome formation from subunits studied by stopped-flow and Rayleigh light scattering
Directory of Open Access Journals (Sweden)
Antoun Ayman
2004-01-01
Full Text Available Light scattering and standard stopped-flow techniques were used to monitor rapid association of ribosomal subunits during initiation of eubacterial protein synthesis. The effects of the initiation factors IF1, IF2, IF3 and buffer conditions on subunit association were studied along with the role of GTP in this process. The part of light scattering theory that is essential for kinetic measurements is high-lighted in the main text and a more general treatment of Rayleigh scattering from macromolecules is given in an appendix.
Yang, Xiaodong
The strong light localization and long photon lifetimes in two-dimensional silicon photonic crystal nanocavities with high quality factor (Q ) and subwavelength modal volume (V) significantly enhance the light-matter interactions, presenting many opportunities to explore new functionalities in silicon nanophotonic integrated circuits for on-chip all-optical information processing, optical computation and optical communications. This thesis will focus on the design, nanofabrication, and experimental characterization of both passive and active silicon nanophotonic devices based on two-dimensional high-Q silicon photonic crystal nanocavities. Three topics of controlling light with these high-Q nanocavities will be presented, including (1) photon confinement mechanism and cavity resonance tuning, (2) enhancement of optical nonlinearities, and (3) all-optical analogue to coherent interferences. The first topic is photon confinement in two-dimensional high- Q silicon photonic crystal nanocavities. In Chapter 2, the role of Q/V as the figure of merit for the enhanced light-matter interaction in optical microcavities and nanocavities is explained and different types of high-Q optical microcavities and nanocavities are reviewed with an emphasis on two-dimensional photonic crystal nanocavities. Then the nanofabrication process and the Q characterization are illustrated for the two-dimensional silicon photonic crystal nanocavities. In Chapter 3, the post-fabrication digital resonance tuning of high-Q silicon photonic crystal nanocavities using atomic layer deposition is proposed and demonstrated, with wide tuning range and precise control of cavity resonances while preserving high quality factors. The second topic is the enhancement of optical nonlinearities in two-dimensional high-Q silicon photonic crystal nanocavities, including stimulated Raman scattering and thermo-optical nonlinearities. In Chapter 4, the enhanced stimulated Raman scattering for low threshold Raman
Non-Linear Compton Scattering of Ultrashort and Ultraintense Laser Pulses
Seipt, D
2010-01-01
The scattering of temporally shaped intense laser pulses off electrons is discussed by means of manifestly covariant quantum electrodynamics. We employ a framework based on Volkov states with a time dependent laser envelope in light-cone coordinates within the Furry picture. An expression for the cross section is constructed, which is independent of the considered pulse shape and pulse length. A broad distribution of scatted photons with a rich pattern of subpeaks like that obtained in Thomson scattering is found. These broad peaks may overlap at sufficiently high laser intensity, rendering inappropriate the notion of individual harmonics. The limit of monochromatic plane waves as well as the classical limit of Thomson scattering are discussed. As a main result, a scaling law is presented connecting the Thomson limit with the general result for arbitrary kinematics. In the overlapping regions of the spectral density, the classical and quantum calculations give different results, even in the Thomson limit. Thu...
The optimal antenna for nonlinear spectroscopy of weakly and strongly scattering nanoobjects
Schumacher, Thorsten; Brandstetter, Matthias; Wolf, Daniela; Kratzer, Kai; Hentschel, Mario; Giessen, Harald; Lippitz, Markus
2016-04-01
Optical nanoantennas, i.e., arrangements of plasmonic nanostructures, promise to enhance the light-matter interaction on the nanoscale. In particular, nonlinear optical spectroscopy of single nanoobjects would profit from such an antenna, as nonlinear optical effects are already weak for bulk material, and become almost undetectable for single nanoobjects. We investigate the design of optical nanoantennas for transient absorption spectroscopy in two different cases: the mechanical breathing mode of a metal nanodisk and the quantum-confined carrier dynamics in a single CdSe nanowire. In the latter case, an antenna with a resonance at the desired wavelength optimally increases the light intensity at the nanoobject. In the first case, the perturbation of the antenna by the investigated nanosystem cannot be neglected and off-resonant antennas become most efficient.
Analysis of Light Scattering by Nanoobjects on a Plane Surface via Discrete Sources Method
Eremina, Elena; Eremin, Yuri; Wriedt, Thomas
2012-12-01
In the last years light scattering by nanostructures is of interest in different areas of science and technology. Analysis of light scattered by nanostructures is an effective tool for a better understanding of their properties. In this work the Discrete Sources Method (DSM) is applied to model light scattering by nanoparticles on a surface. One of attractive features of the DSM is an ability to account for all the features of the modeled system, such as complex refractive index with frequency dispersion of particles and a substrate, scattering interaction of particle and an interface. To demonstrate the variety of possible applications for the DSM, we concentrated on two practical applications. First is light scattering by a nanorod on a surface, which requires the use of a general 3D version of the DSM. The second case discussed in this chapter is light scattering by a nanoshell, which allows the accounting for the axial symmetry of the problem and essential reduction of calculation time. In both cases light scattering characteristics and their dependence on nanostructure characteristics like size, symmetry, incident angle, particle orientation, refractive index and wavelength are analyzed and discussed.
Polarized light scattering as a probe for changes in chromosome structure
Energy Technology Data Exchange (ETDEWEB)
Shapiro, Daniel Benjamin [Univ. of California, Berkeley, CA (United States)
1993-10-01
Measurements and calculations of polarized light scattering are applied to chromosomes. Calculations of the Mueller matrix, which completely describes how the polarization state of light is altered upon scattering, are developed for helical structures related to that of chromosomes. Measurements of the Mueller matrix are presented for octopus sperm heads, and dinoflagellates. Comparisons of theory and experiment are made. A working theory of polarized light scattering from helices is developed. The use of the first Born approximation vs the coupled dipole approximation are investigated. A comparison of continuous, calculated in this work, and discrete models is also discussed. By comparing light scattering measurements with theoretical predictions the average orientation of DNA in an octopus sperm head is determined. Calculations are made for the Mueller matrix of DNA plectonemic helices at UV, visible and X-ray wavelengths. Finally evidence is presented that the chromosomes of dinoflagellates are responsible for observed differential scattering of circularly-polarized light. This differential scattering is found to vary in a manner that is possibly correlated to the cell cycle of the dinoflagellates. It is concluded that by properly choosing the wavelength probe polarized light scattering can provide a useful tool to study chromosome structure.
Scattering of Sculpted Light in Intact Brain Tissue, with implications for Optogenetics
Favre-Bulle, Itia A.; Preece, Daryl; Nieminen, Timo A.; Heap, Lucy A.; Scott, Ethan K.; Rubinsztein-Dunlop, Halina
2015-06-01
Optogenetics uses light to control and observe the activity of neurons, often using a focused laser beam. As brain tissue is a scattering medium, beams are distorted and spread with propagation through neural tissue, and the beam’s degradation has important implications in optogenetic experiments. To address this, we present an analysis of scattering and loss of intensity of focused laser beams at different depths within the brains of zebrafish larvae. Our experimental set-up uses a 488 nm laser and a spatial light modulator to focus a diffraction-limited spot of light within the brain. We use a combination of experimental measurements of back-scattered light in live larvae and computational modelling of the scattering to determine the spatial distribution of light. Modelling is performed using the Monte Carlo method, supported by generalised Lorenz-Mie theory in the single-scattering approximation. Scattering in areas rich in cell bodies is compared to that of regions of neuropil to identify the distinct and dramatic contributions that cell nuclei make to scattering. We demonstrate the feasibility of illuminating individual neurons, even in nucleus-rich areas, at depths beyond 100 μm using a spatial light modulator in combination with a standard laser and microscope optics.
Luk`yanchuk, Boris S; Paniagua-Dominguez, Ramon; Kuznetsov, Arseniy I
2014-01-01
High-refractive index dielectric nanoparticles may exhibit strong directional forward light scattering at visible and near-infrared wavelengths due to interference of simultaneously excited electric and magnetic dipole resonances. For a spherical high-index dielectric, the so-called first Kerker's condition can be realized, at which the backward scattering practically vanishes for some combination of refractive index and particle size. However, Kerker's condition for spherical particles is only possible at the tail of the scattering resonances, when the particle scatters light weakly. Here we demonstrate that significantly higher forward scattering can be realized if spheroidal particles are considered instead. For each value of refractive index exists an optimum shape of the particle, which produces minimum backscattering efficiency together with maximum forward scattering. This effect is achieved due to the overlapping of magnetic and electric dipole resonances of the spheroidal particle at the resonance fr...
Light scattering by a spherical particle with multiple densely packed inclusions
Institute of Scientific and Technical Information of China (English)
Sun Xian-Ming; Wang Hai-Hua; Liu Wan-Qiang; Shen Ji
2009-01-01
This paper calculates light scattering by a spherical water particle containing densely packed inclusions at a visible wavelength 0.55 μm by a combination of ray-tracing and Monte Carlo techniques. While the individual reflection and refraction events at the outer boundary of a sphere particle are considered by a ray-tracing program, the Monte Carlo routine simulates internal scattering processes. The main advantage of this method is that the shape of the particle can be arbitrary, and multiple scattering can be considered in the internal scattering processes. A dense-medium light-scattering theory based on the introduction of the static structure factor is used to calculate the phase function and asymmetry parameters for densely packed inclusions. Numerical results of the single scattering characteristics for a sphere containing multiple densely packed inclusions are given.
Density of states governs light scattering in photonic crystals
García, P D; Froufe-Pérez, Luis S; López, C
2008-01-01
We describe a smooth transition from (fully ordered) photonic crystal to (fully disordered) photonic glass that enables us to make an accurate measurement of the scattering mean free path in nanostructured media and, in turn, establishes the dominant role of the density of states. We have found one order of magnitude chromatic variation in the scattering mean free path in photonic crystals for just $\\sim 3%$ shift around the band-gap ($\\sim 27$ nm in wavelength).
Ulku, Huseyin Arda
2014-07-06
Effects of material nonlinearities on electromagnetic field interactions become dominant as field amplitudes increase. A typical example is observed in plasmonics, where highly localized fields “activate” Kerr nonlinearities. Naturally, time domain solvers are the method of choice when it comes simulating these nonlinear effects. Oftentimes, finite difference time domain (FDTD) method is used for this purpose. This is simply due to the fact that explicitness of the FDTD renders the implementation easier and the material nonlinearity can be easily accounted for using an auxiliary differential equation (J.H. Green and A. Taflove, Opt. Express, 14(18), 8305-8310, 2006). On the other hand, explicit marching on-in-time (MOT)-based time domain integral equation (TDIE) solvers have never been used for the same purpose even though they offer several advantages over FDTD (E. Michielssen, et al., ECCOMAS CFD, The Netherlands, Sep. 5-8, 2006). This is because explicit MOT solvers have never been stabilized until not so long ago. Recently an explicit but stable MOT scheme has been proposed for solving the time domain surface magnetic field integral equation (H.A. Ulku, et al., IEEE Trans. Antennas Propag., 61(8), 4120-4131, 2013) and later it has been extended for the time domain volume electric field integral equation (TDVEFIE) (S. B. Sayed, et al., Pr. Electromagn. Res. S., 378, Stockholm, 2013). This explicit MOT scheme uses predictor-corrector updates together with successive over relaxation during time marching to stabilize the solution even when time step is as large as in the implicit counterpart. In this work, an explicit MOT-TDVEFIE solver is proposed for analyzing electromagnetic wave interactions on scatterers exhibiting Kerr nonlinearity. Nonlinearity is accounted for using the constitutive relation between the electric field intensity and flux density. Then, this relation and the TDVEFIE are discretized together by expanding the intensity and flux - sing half
Shcherbakov, A S; Arellanes, A O; Chavushyan, V
2016-12-01
We develop an advanced approach to the optical spectrometer with acousto-optical dynamic grating for the Guillermo Haro astrophysical observatory (Mexico). The progress consists of two principle novelties. First is the use of the acousto-optical nonlinearity of two-phonon light scattering in crystals with linear acoustic losses. This advanced regime of light scattering exhibits a recently revealed additional degree of freedom, which allows tuning of the frequency of elastic waves and admits the nonlinear apodization improving the dynamic range. The second novelty is the combination of the cross-disperser with acousto-optical processing. A similar pioneering step provides an opportunity to operate over all the visible range in a parallel regime with maximal achievable resolution. The observation window of the optical spectrometer in that observatory is ∼9 cm, so that the theoretical estimations of maximal performances for a low-loss LiNbO3 crystal for this optical aperture at λ=405 nm give spectral resolution of 0.0523 Å, resolving power of 77,400, and 57,500 spots. The illustrative proof-of-principle experiments with a 6 cm LiNbO3 crystal have been performed.
Rapoport, Yu G.; Boardman, A. D.; Grimalsky, V. V.; Ivchenko, V. M.; Kalinich, N.
2014-05-01
The idea of nonlinear ‘transformation optics-inspired’ [1-6] electromagnetic cylindrical field concentrators has been taken up in a preliminary manner in a number of conference reports [7-9]. Such a concentrator includes both external linear region with a dielectric constant increased towards the centre and internal region with nonlinearity characterized by constant coefficients. Then, in the process of farther investigations we realized the following factors considered neither in [7-9] nor in the recent paper [10]: saturation of nonlinearity, nonlinear losses, linear gain, numerical convergence, when nonlinear effect becomes very strong and formation of ‘hotspots’ starts. It is clearly demonstrated here that such a strongly nonlinear process starts when the nonlinear amplitude of any incident beam(s) exceeds some ‘threshold’ value. Moreover, it is shown that the formation of hotspots may start as the result of any of the following processes: an increase of the input amplitude, increasing the linear amplification in the central nonlinear region, decreasing the nonlinear losses, a decrease in the saturation of the nonlinearity. Therefore, a tendency to a formation of ‘hotspots’ is a rather universal feature of the strongly nonlinear behaviour of the ‘nonlinear resonator’ system, while at the same time the system is not sensitive to the ‘prehistory’ of approaching nonlinear threshold intensity (amplitude). The new proposed method includes a full-wave nonlinear solution analysis (in the nonlinear region), a new form of complex geometric optics (in the linear inhomogeneous external cylinder), and new boundary conditions, matching both solutions. The observed nonlinear phenomena will have a positive impact upon socially and environmentally important devices of the future. Although a graded-index concentrator is used here, it is a direct outcome of transformation optics. Numerical evaluations show that for known materials these nonlinear effects
Jiao, J. P.; Drinkwater, B. W.; Neild, S. A.; Wilcox, P. D.
2009-06-01
Guided wave structural health monitoring offers the prospect of continuous interrogation of large plate-like structures with a sparse network of permanently attached sensors. Currently, the most common approach is to monitor changes in the received signals by subtraction from a reference signal obtained when the structure was known to be defect-free. In this paper a comparison is made between this defect-free subtraction approach and a technique in which low-frequency vibration modulation of guided wave signals is used to detect nonlinear scatterers. The modulation technique potentially overcomes the need for the defect-free reference measurement as the subtraction is now made between different parts of an externally applied low-frequency vibration. Linear defects were simulated by masses bonded onto a plate and nonlinear scatterers were simulated by loading a similar mass against the plate. The experimental results show that the defect-free subtraction technique performs well in detecting the bonded mass whereas the modulation technique is able to discriminate between the bonded and loaded masses. Furthermore, because the modulation technique does not require a defect-free reference, it is shown to be relatively independent of temperature effects, a significant problem for reference based subtraction techniques.
Validation of in-line surface characterization by light scattering in Robot Assisted Polishing
DEFF Research Database (Denmark)
Pilny, Lukas; Bissacco, Giuliano; De Chiffre, Leonardo
2014-01-01
The suitability of a commercial scattered light sensor for in-line characterization of fine surfaces in the roughness range Sa 1 – 30 nm generated by the Robot Assisted Polishing (RAP) was investigated and validated. A number of surfaces were generated and directly measured with the scattered lig...
Dynamics of spontaneous radiation of atoms scattered by a resonance standing light wave
Fedorov, MV; Efremov, MA; Yakovlev, VP; Schleich, WP
2003-01-01
The scattering of atoms by a resonance standing light wave is considered under conditions when the lower of two resonance levels is metastable, while the upper level rapidly decays due to mainly spontaneous radiative transitions to the nonresonance levels of an atom. The diffraction scattering regim
Formation of liquid inclusion induced light scatter in KDP (DKDP) crystals
Institute of Scientific and Technical Information of China (English)
孙洵; 孙大亮; 许心光; 王正平; 付有君; 王圣来; 曾红; 李毅平; 于锡玲; 高樟寿
2001-01-01
We describe in this paper the formation of liquid inclusion induced light scatter in potassium dihydrogen phosphate (KDP) crystal and deuterated potassium dihydrogen phosphate (DKDP) crystals. The measurement has been done with an atomic force microscope (AFM). The mechanism of formation of liquid inclusion scatter has been proposed and the effect of super-saturation discussed.
Energy Technology Data Exchange (ETDEWEB)
Dishman, K.L.; Doolin, P.K.; Hoffman, J.F. (Ashland Petroleum Co., Ashland, KY (United States))
1993-07-01
A method of interconversion of dry sieve and laser light scattering particle size values has been developed for cracking catalysts. Values obtained by light scattering techniques were consistently larger than those obtained by dry sieve analysis. The differences were primarily due to lack of sphericity of the particles. The particle size distribution determined by light scattering techniques was based on an average particle diameter. Conversely, the sieve measured the smallest diameter of the particle which can pass through the opening. Microscopic examination of commercial cracking catalysts confirmed their nonuniformity. The sphericity of the catalyst particles decreased as particle size increased. Therefore, the divergence between the laser light scattering and dry sieving value became greater as the catalyst particle size increased.
Kokhanovsky, Alexander A
2014-01-01
This book describes modern advances in radiative transfer and light scattering. Coverage includes fast radiative transfer techniques, use of polarization in remote sensing and recent developments in remote sensing of snow properties from space observations.
Light Scattering and Thermal Emission by Primitive Dust Particles in Planetary Systems
Kimura, Hiroshi; Li, Aigen; Lebreton, Jérémy
2016-01-01
This review focuses on numerical approaches to deducing the light-scattering and thermal-emission properties of primitive dust particles in planetary systems from astronomical observations. The particles are agglomerates of small grains with sizes comparable to visible wavelength and compositions being mainly magnesium-rich silicates, iron-bearing metals, and organic refractory materials in pristine phases. These unique characteristics of primitive dust particles reflect their formation and evolution around main-sequence stars of essentially solar composition. The development of light-scattering theories has been offering powerful tools to make a thorough investigation of light scattering and thermal emission by primitive dust agglomerates in such a circumstellar environment. In particular, the discrete dipole approximation, the T-matrix method, and effective medium approximations are the most popular techniques for practical use in astronomy. Numerical simulations of light scattering and thermal emission by ...
Neutron and photon (light) scattering on solitons in the quasi-one-dimensional magnetics
Abdulloev, K O
1999-01-01
The general expression we have found earlier for the dynamics form-factor is used to analyse experiments on the neutron and photon (light) scattering by the gas of solitons in quasi-one-dimensional magnetics (Authors)
Energy Technology Data Exchange (ETDEWEB)
Sorensen, C.M.
1976-01-01
An effort to expand light-scattering autocorrelation techniques to Brownian diffusional and critical fluid systems in which multiple scattering effects are important, and to understand the observed similarity of the Rayleigh linewidth of light scattered from these two seemingly different systems is discussed. A formalism was developed to find the light field multiply scattered from a suspension of Brownian diffusing particles. For the field doubly scattered from a system of noninteracting Brownian particles, the intensity and correlation time were much less dependent on the scattering angle than for the singly scattered component. The polarized and depolarized correlation times of light scattered from Brownian particle systems were measured. The double-scattering formalism was extended to light scattered from critical fluid systems. In the region k xi greater than 5 the doubly and singly scattered correlation times were nearly equal. The dynamic droplet model of critical phenomena was developed which gives the proper, experimentally verified, forms for the intensity and linewidth of light scattered from a critical fluid. To test the dynamic droplet model and the mode theories Rayleigh linewidth predictions, light-scattering measurements were performed on the critical fluid system methanol and cyclohexane. The data agreed with both the dynamic droplet and decoupled mode theory predictions. The depolarized scattered spectra from a critical fluid were measured, and qualitative agreement with the double-scattering theory was found. 57 figures, 5 tables.
The scatter of light of different colour in the atmosphere.
Schreuder, D.A.
1976-01-01
It is often claimed (Devaux) that yellow light is superior to white light for vehicle headlamps. This claim is supported by evidence of a physical, physiological and psychological nature. In most cases, it appears that the advantages of yellow light are small, and can usually be neglected particul
Simplifying the calculation of light scattering properties for black carbon fractal aggregates
Directory of Open Access Journals (Sweden)
A. J. A. Smith
2014-02-01
Full Text Available Black carbon fractal aggregates have complicated shapes that make the calculation of their optical properties particularly computationally expensive. Here, a method is presented to estimate fractal aggregate light scattering properties by optimising simplified models to full light scattering calculations. It is found that there are no possible spherical models (at any size or refractive index that well represent the light scattering in the visible, or near-thermal infrared. As such, parameterisations of the light scattering as a function of the number of aggregate particles is presented as the most pragmatic choice for modelling distributions of black carbon when the large computational overheads of rigorous scattering calculations cannot be justified. This parameterisation can be analytically integrated to provide light scattering properties for log-normal distributions of black carbon fractal aggregates and return extinction cross-sections with 0.1% accuracy for typical black carbon size distributions. Scattering cross-sections and the asymmetry parameter can be obtained to within 3%.
Optical Imaging of Cells with Gold Nanoparticle Clusters as Light Scattering Contrast Agents
DEFF Research Database (Denmark)
Tanev, Stoyan
2011-01-01
developments in advanced cytometry research by pointing out potential new research directions. A brief description of the FDTD method focusing on the features associated with its application to modeling of light scattering and OPCM cell imaging experiments is provided. The examples include light scattering...... from OPCM imaging of single biological cells in conditions of controlled refractive index matching (RIM) and labeling by diffused and clustered gold NPs. The chapter concludes with a discussion and suggestions for future research....
T-matrix computations of light scattering by red blood cells
Nilsson, Annika M. K.; Alsholm, Peter; Karlsson, Anders; Andersson-Engels, Stefan
1998-01-01
The electromagnetic far field, as well as near field, originating from light interaction with a red blood cell (RBC) volume equivalent spheroid, were analyzed utilizing T-matrix theory. This method is a powerful tool which enables the influence of cell shape on the angular distribution of scattered light to be studied. General observations were that the three-dimensional shape, as well as optical thickness apparent to the incident field, affect the forward scattering. The ba...
Zhou, Xiaoji; Xu, Xu; Yin, Lan; Liu, W M; Chen, Xuzong
2010-07-19
We propose a new method of detecting quantum coherence of a Bose gas trapped in a one-dimensional optical lattice by measuring the light intensity from Raman scattering in cavity. After pump and displacement process, the intensity or amplitude of scattering light is different for different quantum states of a Bose gas, such as superfluid and Mott-Insulator states. This method can also be useful to detect quantum states of atoms with two components in an optical lattice.
Measurement-Induced Strong Kerr Nonlinearity for Weak Quantum States of Light
Costanzo, Luca S.; Coelho, Antonio S.; Biagi, Nicola; Fiurášek, Jaromír; Bellini, Marco; Zavatta, Alessandro
2017-07-01
Strong nonlinearity at the single photon level represents a crucial enabling tool for optical quantum technologies. Here we report on experimental implementation of a strong Kerr nonlinearity by measurement-induced quantum operations on weak quantum states of light. Our scheme coherently combines two sequences of single photon addition and subtraction to induce a nonlinear phase shift at the single photon level. We probe the induced nonlinearity with weak coherent states and characterize the output non-Gaussian states with quantum state tomography. The strong nonlinearity is clearly witnessed as a change of sign of specific off-diagonal density matrix elements in the Fock basis.
Directory of Open Access Journals (Sweden)
H.-C. Wu (武慧春
2011-07-01
Full Text Available A new way to generate intense attosecond x-ray pulses is discussed. It relies on coherent Thomson scattering (CTS from relativistic electron sheets. A double layer technique is used to generate planar solid-density sheets of monochromatic high-γ electrons with zero transverse momentum such that coherently backscattered light is frequency upshifted by factors up to 4γ^{2}. Here previous work [H.-C. Wu et al., Phys. Rev. Lett. 104, 234801 (2010PRLTAO0031-900710.1103/PhysRevLett.104.234801] is extended to the regime of high-intensity probe light with normalized amplitude a_{0}>1 leading to nonlinear CTS effects such as pulse contraction and steepening. The results are derived both by particle-in-cell (PIC simulation in a boosted frame and by analytic theory. PIC simulation shows that powerful x-ray pulses (1 keV, 10 gigawatt can be generated. They call for experimental verification. Required prerequisites such as manufacture of nanometer-thick target foils is ready and ultrahigh contrast laser pulses should be within reach in the near future.
Anomalous Light Scattering by Topological PT-symmetric Particle Arrays
Ling, C. W.; Choi, Ka Hei; Mok, T. C.; Zhang, Zhao-Qing; Fung, Kin Hung
2016-12-01
Robust topological edge modes may evolve into complex-frequency modes when a physical system becomes non-Hermitian. We show that, while having negligible forward optical extinction cross section, a conjugate pair of such complex topological edge modes in a non-Hermitian -symmetric system can give rise to an anomalous sideway scattering when they are simultaneously excited by a plane wave. We propose a realization of such scattering state in a linear array of subwavelength resonators coated with gain media. The prediction is based on an analytical two-band model and verified by rigorous numerical simulation using multiple-multipole scattering theory. The result suggests an extreme situation where leakage of classical information is unnoticeable to the transmitter and the receiver when such a -symmetric unit is inserted into the communication channel.
Nonlinear kinetic modeling of stimulated Raman scattering in a multidimensional geometry
Energy Technology Data Exchange (ETDEWEB)
Benisti, D.; Morice, O.; Gremillet, L.; Friou, A.; Lefebvre, E. [CEA, DAM, DIF F-91297 Arpajon (France)
2012-05-15
In this paper, we derive coupled envelope equations modeling the growth of stimulated Raman scattering (SRS) in a multi-dimensional geometry and accounting for nonlinear kinetic effects. In particular, our envelope equations allow for the nonlinear reduction of the Landau damping rate, whose decrease with the plasma wave amplitude depends on the rate of side-loss. Account is also made of the variations in the extent of the plasma wave packet entailed by the collisionless dissipation due to trapping. The dephasing between the electron plasma wave (EPW) and the laser drive, as well as the self-focussing of the plasma wave, both induced by the EPW nonlinear frequency shift, are also included in our envelope equations. These equations are solved in a multi-dimensional geometry using our code dubbed BRAMA, whose predictions regarding the evolution of Raman reflectivity as a function of the laser intensity are compared against previously published particle in cell results, thus illustrating the ability of BRAMA simulations to provide the correct laser threshold intensity for SRS as well as the right order of magnitude of Raman reflectivity above threshold.
Ochirbat, G
2000-01-01
A plane medium, whose dielectric tensor's principal values arbitrarily depend upon intensity, is considered. The problems of the TM and TE waves, within the problem of light scattering, are reduced to quadrature. A question of integrability of the full system of Maxwell equations is discussed. A closed equation has been obtained for an auxiliary variable for a nonlinearity of Kerr type. A scheme for integrating the full system of Maxwell equations by solving the equation over the auxiliary variable is suggested.
Directory of Open Access Journals (Sweden)
Manvir S. Kushwaha
2012-09-01
Full Text Available The most fundamental approach to an understanding of electronic, optical, and transport phenomena which the condensed matter physics (of conventional as well as nonconventional systems offers is generally founded on two experiments: the inelastic electron scattering and the inelastic light scattering. This work embarks on providing a systematic framework for the theory of inelastic electron scattering and of inelastic light scattering from the electronic excitations in GaAs/Ga1−xAlxAs quantum wells. To this end, we start with the Kubo's correlation function to derive the generalized nonlocal, dynamic dielectric function, and the inverse dielectric function within the framework of Bohm-Pines’ random-phase approximation. This is followed by a thorough development of the theory of inelastic electron scattering and of inelastic light scattering. The methodological part is then subjected to the analytical diagnoses which allow us to sense the subtlety of the analytical results and the importance of their applications. The general analytical results, which know no bounds regarding, e.g., the subband occupancy, are then specified so as to make them applicable to practicality. After trying and testing the eigenfunctions, we compute the density of states, the Fermi energy, the full excitation spectrum made up of intrasubband and intersubband – single-particle and collective (plasmon – excitations, the loss functions for all the principal geometries envisioned for the inelastic electron scattering, and the Raman intensity, which provides a measure of the real transitions induced by the (laser probe, for the inelastic light scattering. It is found that the dominant contribution to both the loss peaks and the Raman peaks comes from the collective (plasmon excitations. As to the single-particle peaks, the analysis indicates a long-lasting lack of quantitative comparison between theory and experiments. It is inferred that the inelastic electron
Coherent anti-Stokes Raman scattering microscopy with a photonic crystal fiber based light source
DEFF Research Database (Denmark)
Paulsen, H.N.; Hilligsøe, Karen Marie; Thøgersen, J.
2003-01-01
A coherent anti-Stokes Raman scattering microscope based on a Ti:sapphire femtosecond oscillator and a photonic crystal fiber is demonstrated. The nonlinear response of the fiber is used to generate the additional wavelength needed in the Raman process. The applicability of the setup is demonstra...... is demonstrated by imaging of micrometer-sized polystyrene beads....
Coupled force-balance and scattering equations for nonlinear transport in quantum wires
Huang, Danhong; Gumbs, Godfrey
2009-07-01
The coupled force-balance and scattering equations have been derived and applied to study nonlinear transport of electrons subjected to a strong dc electric field in an elastic-scattering-limited quantum wire. Numerical results have demonstrated both field-induced heating-up and cooling-down behaviors in the nonequilibrium part of the total electron-distribution function by varying the impurity density or the width of the quantum wire. The obtained asymmetric distribution function in momentum space invalidates the application of the energy-balance equation to our quantum-wire system in the center-of-mass frame. The experimentally observed suppression of mobility by a driving field for the center-of-mass motion in the quantum-wire system has been reproduced [see K. Tsubaki , Electr. Lett. 24, 1267 (1988); M. Hauser , Sci. Technol. 9, 951 (1994)]. In addition, the thermal enhancement of mobility in the elastic-scattering-limited system has been demonstrated, in accordance with a similar prediction made for graphene nanoribbons [see T. Fang , Phys. Rev. B 78, 205403 (2008)]. This thermal enhancement has been found to play a more and more significant role with higher lattice temperature and becomes stronger for a low-driving field.
Indian Academy of Sciences (India)
Hari Prakash; Devendra K Singh
2010-03-01
It is shown that all optical polarization states of light except plane and circular polarization states undergo an intensity-dependent change in normal incidence of light in an isotropic nonlinear Kerr medium. This effect should be detectable and we propose an experiment for detecting nonlinear susceptibility involved in that part of nonlinear polarization, which depends on the polarization state of light also.
Bienaime, Tom; Chabe, Julien; Rouabah, Mohamed-Taha; Bellando, Louis; Courteille, Philippe W; Piovella, Nicola; Kaiser, Robin
2013-01-01
The interplay between the superradiant emission of a cloud of cold two-level atoms and the radiation pressure force is discussed. Using a microscopic model of coupled atomic dipoles driven by an external laser, the radiation field and the average radiation pressure force are derived. A relation between the far-field scattered intensity and the force is derived, using the optical theorem. Finally, the scaling of the sample scattering cross section with the parameters of the system is studied.
Gogoi, Ankur
Light scattering is a subject of intensive research at the present time in diverse fields of research namely, physics, astronomy, meteorology, biology, nanotechnology, etc. Observation and theoretical calculation of the absorption and scattering properties of particles, whose size ranges from micrometer to nanometer, are not only essential to deduce their physical properties but also capable of giving useful information for better understanding of radiation transfer through a medium containing such scatterer. In addition to such experimental and theoretical studies on light scattering by particulate matter several other groups have been extensively using Monte Carlo (MC) method to simulate light (photon) propagation in scattering media. Importantly such methods of simulating light scattering properties of artificial particles are proving to be a very useful tool in verifying the experimental observations with real samples as well as providing new clues to improve the accuracy of the existing theoretical models. In this contribution we report a MC method developed by implementing Mie theory to simulate the light scattering pattern from size distributed homogenous and coated spherical particles in single scattering regime. The computer program was written in ANSI C-language. The accuracy, efficiency and reliability of the MC method were validated by comparing the results generated by using the MC method with other benchmark theoretical results and experimental results with standard samples. Notably the MC method reported here is found to be stable even for very large spherical particles (size parameters > 1000) with large values of real (= 10) and imaginary part (= 10) of the refractive index. The promising field of application of the reported MC method will be in simulating the light (or electromagnetic) scattering properties of different types of planetary and interplanetary dust particles.
Shahin, Hesam; Gupta, Manisha; Janowska-Wieczorek, Anna; Rozmus, Wojciech; Tsui, Ying Y
2016-12-12
An experimental setup capable of measuring simultaneous 2D scattered light angular distribution from two directions to study cell morphology without the use of bio-labels was developed. Experiments with hematopoietic stem cells (CD34+ cells) show good agreement with detailed numerical simulations of light scattering. Numerical simulations and computer models of cells are used to identify physical features of cells with the largest scattering cross sections. This allows for determination of size, geometry of the nucleus and distribution of mitochondria in hematopoietic stem cells by means of our label-free method.
Imaging in scattering media via the second-order correlation of light field
Gong, Wenlin; Shen, Xia; Han, Shensheng
2009-01-01
Imaging with the second-order correlation of two light fields is a method to image an object by two-photon interference involving a joint detection of two photons at distant space-time points. We demonstrate for the first time that an image with high quality can still be obtained in the scattering media by applying the second-order correlation of illuminating light field. The scattering effect on the visibility of images is analyzed both theoretically and experimentally. Potential applications and the methods to further improve the visibility of the images in scattering media are also discussed.
Double scattering of light from biophotonic nanostructures with short-range order
Noh, Heeso; Saranathan, Vinodkumar; Prum, Richard O; Mochrie, Simon G J; Dufresne, Eric R; Cao, Hui
2009-01-01
We investigate the physical mechanism for color production by isotropic nanostructures with short-range order in bird feather barbs. While the primary peak in optical scattering spectra results from constructive interference of singly-scattered light, many species exhibit secondary peaks with distinct characteristic. Our experimental and numerical studies show that these secondary peaks result from double scattering of light by the correlated structures. Without an analog in periodic or random structures, such a phenomenon is unique for short-range ordered structures, and has been widely used by nature for non-iridescent structural coloration.
Experimental demonstration of singular-optical colouring of regularly scattered white light
DEFF Research Database (Denmark)
Angelsky, O.V.; Hanson, Steen Grüner; Maksimyak, P.P.
2008-01-01
Experimental interference modelling of the effects of colouring of a beam traversing a light-scattering medium is presented. It is shown that the result of colouring of the beam at the output of the medium depends on the magnitudes of the phase delays of the singly forward scattered partial signals....... The colouring mechanism has for the first time experimentally been illustrated for a forward propagating beam through a light-scattering medium. This is showed in video-fragments of the interferograms recorded within the zero interference fringe with a gradual change of the path difference of the interfering...
Optimal control of light propagation through multiple-scattering media in the presence of noise
Yilmaz, Hasan; Mosk, Allard P
2013-01-01
We study the control of coherent light propagation through multiple-scattering media in the presence of measurement noise. In our experiments, we use a two-step optimization procedure to find the optimal incident wavefront. We conclude that the degree of optimal control of coherent light propagation through a multiple-scattering medium is only determined by the number of photoelectrons detected per single speckle spot. The prediction of our model agrees well with the experimental results. Our results offer opportunities for imaging applications through scattering media such as biological tissue in the shot noise limit.
Observation of spatial quantum correlations induced by multiple scattering of nonclassical light.
Smolka, S; Huck, A; Andersen, U L; Lagendijk, A; Lodahl, P
2009-05-15
We present the experimental realization of spatial quantum correlations of photons that are induced by multiple scattering of squeezed light. The quantum correlation relates photons propagating along two different light paths through the random medium and is infinite in range. Both positive and negative spatial quantum correlations are observed when varying the quantum state incident to the multiple scattering medium, and the strength of the correlations is controlled by the number of photons. The experimental results are in excellent agreement with recent theoretical proposals by implementing the full quantum model of multiple scattering.
Microchip Flow Cytometer with Integrated Polymer Optical Elements for Measurement of Scattered Light
DEFF Research Database (Denmark)
Wang, Zhenyu; El-Ali, Jamil; Perch-Nielsen, Ivan Ryberg
2004-01-01
channels to form a complete microchip flow cytometer. All the optical elements, the microfluidic system, and the fiber-to-waveguide couplers were defined in one layer of polymer (SU-8, negative photoresist) by standard photolithography. With only one single mask procedure, all the fabrication and packaging...... processes can be finished in one day. Polystyrene beads were measured in the microchip flow cytometer, and three signals (forward scattering, large angle scattering and extinction) were measured simultaneously for each bead. The average intensities of the forward Scattered light and the incident light...
Auto-correlation Properties of Scattering Light in Ultrasound-modulated Random Media
Institute of Scientific and Technical Information of China (English)
ZHANG Xiqin; XING Da; LIU Ying; MA Shining
2001-01-01
In this paper, the auto-correlation properties of scattering light in random media modulated by ultrasound were studied. The expression of temporal auto-correlation function of scattering light amplitude in the ultrasound-modulated media was presented. The results show that the auto-correlation function is modulated as the ultrasound is introduced into the media and the modulation amplitude decays with correlation time. The influences of ultrasound amplitude, Brownian diffusion coefficient, scattering and absorption coefficients on auto-correlation function were discussed. The auto-correlation imaging of an object hidden in random media was also studied by the use of Monte Carlo simulations.
Wang, Tao; Jiang, Zhenfei; Ji, Xiaoling; Zhao, Daomu
2016-04-01
Spectral shifts and spectral switches of a polychromatic electromagnetic light wave on scattering from an anisotropic semisoft boundary medium are discussed. It is shown that both the property of the incident field and the character of the scattering medium play roles in the change of the spectrum of the far-zone scattered field. It is also shown that the distribution of the far-zone scattered spectrum, including the magnitude of the spectral shift and the direction at which the spectral switch occurs, is rotationally nonsymmetric.
Surface light scattering: integrated technology and signal processing
DEFF Research Database (Denmark)
Lading, L.; Dam-Hansen, C.; Rasmussen, E.
1997-01-01
The miniaturization of surface-scattering instruments for measuring viscoelastic properties is investigated. The concepts are based on the use of holographic optical elements and integrated optics. Compact forms of optics that provide the necessary spatial and angular selections are devised. Four...
Quantum Interference and Entanglement Induced by Multiple Scattering of Light
DEFF Research Database (Denmark)
Ott, Johan Raunkjær; Mortensen, Asger; Lodahl, Peter
2010-01-01
We report on the effects of quantum interference induced by the transmission of an arbitrary number of optical quantum states through a multiple-scattering medium. We identify the role of quantum interference on the photon correlations and the degree of continuous variable entanglement between tw...
Spherically symmetric inhomogeneous bianisotropic media: Wave propagation and light scattering
DEFF Research Database (Denmark)
Novitsky, Andrey; Shalin, Alexander S.; Lavrinenko, Andrei
2017-01-01
We develop a technique for finding closed-form expressions for electromagnetic fields in radially inhomogeneous bianisotropic media, both the solutions of the Maxwell equations and material tensors being defined by the set of auxiliary two-dimensional matrices. The approach is applied to determine...... the scattering cross-sections by spherical particles, the fields inside which correspond to the Airy-exponential waves....
Institute of Scientific and Technical Information of China (English)
LI Hai-Xia; CHENG Chuan-Fu
2011-01-01
@@ We study the light scattering of an orthogonal anisotropic rough surface with secondary most probable slope distribution It is found that the scattered intensity profiles have obvious secondary maxima, and in the direction perpendicular to the plane of incidence, the secondary maxima are oriented in a curve on the observation plane,which is called the orientation curve.By numerical calculation of the scattering wave fields with the height data of the sample, it is validated that the secondary maxima are induced by the side face element, which constitutes the prismoid structure of the anisotropic surface.We derive the equation of the quadratic orientation curve.Experimentally, we construct the system for light scattering measurement using a CCD.The scattered intensity profiles are extracted from the images at different angles of incidence along the orientation curves.The experimental results conform to the theory.
Effects of multiple scattering on light pulses reflected by turbid atmospheres
Weinman, J. A.
1976-01-01
Multiple scattering contributions to lidar returns from turbid atmospheres are derived by means of an analytical theory. It is assumed that scattering takes place mainly at small angles except for one event that scatters the light backward. The phase functions are approximated by the sum of Gaussian functions of the scattering angle in both the forward and backward directions. The three-dimensional radiative transfer equation is transformed to a one-dimensional problem by means of Fourier transforms. Neumann solutions to the transformed equation of radiative transfer are then found. A number of examples are presented for cloud, fog and haze models. The results are found to be in satisfactory agreement with results obtained from the Monte Carlo analysis of Kunkel (1974) and the theory of light pulses doubly scattered by turbid atmospheres which was developed by Eloranta (1972).
The measurement and modelling of light scattering by phytoplankton cells at narrow forward angles
MacCallum, Iain; Cunningham, Alex; McKee, David
2004-07-01
A procedure has been devised for measuring the angular dependence of light scattering from suspensions of phytoplankton cells at forward angles from 0.25° to 8°. The cells were illuminated with a spatially-filtered laser beam and the angular distribution of scattered light measured by tracking a photodetector across the Fourier plane of a collecting lens using a stepper-motor driven stage. The procedure was calibrated by measuring scattering from latex bead suspensions with known size distributions. It was then used to examine the scattering from cultures of the unicellular algae Isochrysis galbana (4 µm × 5 µm), Dunaliella primolecta (6 µm × 7 µm) and Rhinomonas reticulata (5 µm × 11 µm). The results were compared with the predictions of Mie theory. Excellent agreement was obtained for spherical particles. A suitable choice of spherical-equivalent scattering parameters was required to enable reasonable agreement within the first diffraction lobe for ellipsoidal particles.
Dynamic Thomson Scattering from Nonlinear Electron Plasma Waves in a Raman Plasma Amplifier
Davies, A.; Katz, J.; Bucht, S.; Haberberger, D.; Bromage, J.; Zuegel, J. D.; Froula, D. H.; Trines, R.; Bingham, R.; Sadler, J.; Norreys, P. A.
2016-10-01
Electron plasma waves (EPW's) can be used to transfer significant energy from a long-pulse laser to a short-pulse seed laser through the Raman scattering instability. Successful implementation of Raman amplification could open an avenue to producing high-intensity pulses beyond the capabilities of current laser technology ( 1022 W / cm 2). This three-wave interaction takes advantage of the plasma's ability to sustain large-amplitude plasma waves. Having complete knowledge of the EPW amplitude is essential to establishing optimal parameters for high-efficiency Raman amplification. A dynamic Thomson-scattering diagnostic is being developed to spatially and temporally resolve the amplitude of the driven and thermal EPW's. By imaging the scattered probe light onto a novel pulse-front tilt compensated streaked optical spectrometer, the diffraction efficiency of this plasma wave can be measured as a function of space and time. These data will be used in conjunction with particle-in-cell simulations to determine the EPW's spatial and temporal profile. This will allow the effect of the EPW profile on Raman scattering to be experimentally determined. This material is based upon work supported by the Department of Energy National Nuclear Security Administration under Award Number DE-NA0001944.
Statistical-thermodynamic model for light scattering from eye lens protein mixtures
Bell, Michael M.; Ross, David S.; Bautista, Maurino P.; Shahmohamad, Hossein; Langner, Andreas; Hamilton, John F.; Lahnovych, Carrie N.; Thurston, George M.
2017-02-01
We model light-scattering cross sections of concentrated aqueous mixtures of the bovine eye lens proteins γB- and α-crystallin by adapting a statistical-thermodynamic model of mixtures of spheres with short-range attractions. The model reproduces measured static light scattering cross sections, or Rayleigh ratios, of γB-α mixtures from dilute concentrations where light scattering intensity depends on molecular weights and virial coefficients, to realistically high concentration protein mixtures like those of the lens. The model relates γB-γB and γB-α attraction strengths and the γB-α size ratio to the free energy curvatures that set light scattering efficiency in tandem with protein refractive index increments. The model includes (i) hard-sphere α-α interactions, which create short-range order and transparency at high protein concentrations, (ii) short-range attractive plus hard-core γ-γ interactions, which produce intense light scattering and liquid-liquid phase separation in aqueous γ-crystallin solutions, and (iii) short-range attractive plus hard-core γ-α interactions, which strongly influence highly non-additive light scattering and phase separation in concentrated γ-α mixtures. The model reveals a new lens transparency mechanism, that prominent equilibrium composition fluctuations can be perpendicular to the refractive index gradient. The model reproduces the concave-up dependence of the Rayleigh ratio on α/γ composition at high concentrations, its concave-down nature at intermediate concentrations, non-monotonic dependence of light scattering on γ-α attraction strength, and more intricate, temperature-dependent features. We analytically compute the mixed virial series for light scattering efficiency through third order for the sticky-sphere mixture, and find that the full model represents the available light scattering data at concentrations several times those where the second and third mixed virial contributions fail. The model
Stray light analysis for the Thomson scattering diagnostic of the ETE Tokamak
Berni, L. A.; Albuquerque, B. F. C.
2010-12-01
Thomson scattering is a well-established diagnostic for measuring local electron temperature and density in fusion plasma, but this technique is particularly difficult to implement due to stray light that can easily mask the scattered signal from plasma. To mitigate this problem in the multipoint Thomson scattering system implemented at the ETE (Experimento Tokamak Esférico) a detailed stray light analysis was performed. The diagnostic system was simulated in ZEMAX software and scattering profiles of the mechanical parts were measured in the laboratory in order to have near realistic results. From simulation, it was possible to identify the main points that contribute to the stray signals and changes in the dump were implemented reducing the stray light signals up to 60 times.
Sub-Nyquist sampling boosts targeted light transport through opaque scattering media
Shen, Yuecheng; Ma, Cheng; Wang, Lihong V
2016-01-01
Optical time-reversal techniques are being actively developed to focus light through or inside opaque scattering media. When applied to biological tissue, these techniques promise to revolutionize biophotonics by enabling deep-tissue non-invasive optical imaging, optogenetics, optical tweezers and photodynamic therapy. In all previous optical time-reversal experiments, the scattered light field was well-sampled during wavefront measurement and wavefront reconstruction, following the Nyquist sampling criterion. Here, we overturn this conventional practice by demonstrating that even when the scattered field is under-sampled, light can still be focused through or inside opaque media. Even more surprisingly, we show both theoretically and experimentally that the focus achieved by under-sampling is usually about one order of magnitude brighter than that achieved by conventional well-sampling conditions. Moreover, sub-Nyquist sampling improves the signal-to-noise ratio and the collection efficiency of the scattered...
Label-free identification of individual bacteria using Fourier transform light scattering
Jo, YoungJu; Kim, Min-hyeok; Park, HyunJoo; Kang, Suk-Jo; Park, YongKeun
2015-01-01
Rapid identification of bacterial species is crucial in medicine and food hygiene. In order to achieve rapid and label-free identification of bacterial species at the single bacterium level, we propose and experimentally demonstrate an optical method based on Fourier transform light scattering (FTLS) measurements and statistical classification. For individual rod-shaped bacteria belonging to four bacterial species (Listeria monocytogenes, Escherichia coli, Lactobacillus casei, and Bacillus subtilis), two-dimensional angle-resolved light scattering maps are precisely measured using FTLS technique. The scattering maps are then systematically analyzed, employing statistical classification in order to extract the unique fingerprint patterns for each species, so that a new unidentified bacterium can be identified by a single light scattering measurement. The single-bacterial and label-free nature of our method suggests wide applicability for rapid point-of-care bacterial diagnosis.
Stray light analysis for the Thomson scattering diagnostic of the ETE Tokamak
Energy Technology Data Exchange (ETDEWEB)
Berni, L. A. [Instituto Nacional de Pesquisas Espaciais (INPE), Laboratorio Associado de Sensores e Materiais (LAS), 12.227-010 Sao Jose dos Campos, SP (Brazil); Albuquerque, B. F. C. [Instituto Nacional de Pesquisas Espaciais (INPE), Engenharia e Tecnologia Espaciais, Divisao de Eletronica Aeroespacial, 12.227-010 Sao Jose dos Campos, SP (Brazil)
2010-12-15
Thomson scattering is a well-established diagnostic for measuring local electron temperature and density in fusion plasma, but this technique is particularly difficult to implement due to stray light that can easily mask the scattered signal from plasma. To mitigate this problem in the multipoint Thomson scattering system implemented at the ETE (Experimento Tokamak Esferico) a detailed stray light analysis was performed. The diagnostic system was simulated in ZEMAX software and scattering profiles of the mechanical parts were measured in the laboratory in order to have near realistic results. From simulation, it was possible to identify the main points that contribute to the stray signals and changes in the dump were implemented reducing the stray light signals up to 60 times.
Distinguishing Structure Change of Cells Based on Analysis of Light Scattering Patterns
Institute of Scientific and Technical Information of China (English)
JIN Yong-Long; YANG Fang; WANG Meng; ZHANG Yu; GU Ning
2008-01-01
We develop a new method to distinguish structural change of cells based on light scattering and Fourier spectra analysis. The light scattering detection system is composed of a laser source, an optical microscope, a CCD with high resolution and low distortion. After the scattering patterns of cells are recorded by the CCD, the Fourier spectra are obtained by the intensity distribution of scattered light. In the experiment, the change of cell structure is designed by sonication treatment. It is found that different typical peaks can be shown in the Fourier spectra of MCF7 cells with and without sonication treatment, which indicates that this method can be used to distinguish the structural change of cells.
Fluid description of the cooperative scattering of light by spherical atomic clouds
Piovella, N; Courteille, Ph W
2013-01-01
When a cold atomic gas is illuminated by a quasi-resonant laser beam, light-induced dipole-dipole correlations make the scattering of light a cooperative process. Once a fluid description is adopted for the atoms, many scattering properties are captured by the definition of a complex refractive index. The solution of the scattering problem is here presented for spherical atomic clouds of arbitrary density profiles, such as parabolic densities characteristic of ultra-cold clouds. A new solution for clouds with infinite boundaries is derived, that is particularly useful for the Gaussian densities of thermal atomic clouds. The presence of Mie resonances, a signature of the cloud acting as a cavity for the light, is discussed. These resonances leave their fingerprint in various observables such as the scattered intensity or in the radiation pressure force, and can be observed by tuning the frequency of the incident laser field or the atom number.
Elastic scattering and total reaction cross sections with low-energy light radioactive ion beams.
Directory of Open Access Journals (Sweden)
Guimarães Valdir
2011-10-01
Full Text Available Elastic scattering experiments have being performed with low-energy radioactive ion beams produced by the RIBRAS facility in Sao Paulo, Brazil. Here I present the results for elastic scattering of 6He on several targets and light beams on 12C target. Special emphasis is given to the analysis of experiments were angular distributions for the elastic scattering of beryllium isotopes projectiles, 7Be, 9Be and 10Be, on a light target 12C were obtained. These elastic scattering angular distributions have been analysed in terms of optical model using the double-folding Sao Paulo potential. From this analysis, the total reaction cross section were also deduced and compared to the total reaction cross sections for many other light projectiles on 12C target. The comparison was made in terms of Universal Function reduction method.
Dashtdar, Masoomeh; Tavassoly, M Taghi
2009-10-01
We show theoretically and experimentally that the spectrum of coherently scattered light from a randomly rough interface in reflection and transmission is redshifted with a shrinkage in spectral width. In reflection mode the amounts of the redshift and the shrinkage depend on interface roughness, incident angle, and the spectral width of the illuminating light. In transmission mode they also depend on the refractive indices of the surrounding media. The redshift and width shrinkage increase with decrease of the coherently scattered light intensity. This study shows that the spectrum of the diffusely scattered light is blueshifted in the specular direction and in directions with small scattering angles only in situations with appreciable intensity of the coherently scattered light. With decrease of the latter intensity the blueshift reduces and turns into redshift. Also, the redshift and blueshift decay with increase of the scattering angle. An experimental investigation has been carried out, on sheet glasses with different roughness on one side, in reflection and transmission modes. The experimental results and theoretical predictions are quite consistent.
Strokotov, Dmitry I; Moskalensky, Alexander E; Nekrasov, Vyacheslav M; Maltsev, Valeri P
2011-07-01
We instrumentally, theoretically, and experimentally demonstrate a new approach for characterization of nonspherical individual particles from light scattering. Unlike the original optical scheme of the scanning flow cytometer that measures an angle-resolved scattering corresponding in general to S₁₁ element of the light-scattering matrix, the modernized instrument allows us to measure the polarized light-scattering profile of individual particles simultaneously. Theoretically, the polarized profile is expressed by the combination of a few light-scattering matrix elements. This approach supports us with additional independent data to characterize a particle with a complex shape and an internal structure. Applicability of the new method was demonstrated from analysis of polymer bispheres. The bisphere characteristics, sizes, and refractive indices of each sphere composing the bisphere were successfully retrieved from the solution of the inverse light-scattering problem. The solution provides determination of the Eulerian angles, which describe the orientation of the bispheres relative to the direction of the incident laser beam and detecting polarizer of the optical system. Both the ordinary and polarized profiles show a perfect agreement with T-matrix simulation resulting to 50-nm precision for sizing of bispheres. Copyright © 2011 International Society for Advancement of Cytometry.
Winzor, Donald J; Deszczynski, Marcin; Harding, Stephen E; Wills, Peter R
2007-06-01
Experimental data for ovalbumin and lysozyme are presented to highlight the nonequivalence of second virial coefficients obtained for proteins by sedimentation equilibrium and light scattering. Theoretical considerations confirm that the quantity deduced from sedimentation equilibrium distributions is B(22), the osmotic second virial coefficient describing thermodynamic nonideality arising solely from protein self-interaction. On the other hand, the virial coefficient determined by light scattering is shown to reflect the combined contributions of protein-protein and protein-buffer interactions to thermodynamic nonideality of the protein solution. Misidentification of the light scattering parameter as B(22) accounts for published reports of negative osmotic second virial coefficients as indicators of conditions conducive to protein crystal growth. Finally, textbook assertions about the equivalence of second virial coefficients obtained by sedimentation equilibrium and light scattering reflect the restriction of consideration to single-solute systems. Although sedimentation equilibrium distributions for buffered protein solutions are, indeed, amenable to interpretation in such terms, the same situation does not apply to light scattering measurements because buffer constituents cannot be regarded as part of the solvent: instead they must be treated as non-scattering cosolutes.
The propagation dynamics of ultraviolet light filament with Rayleigh scattering in air
Institute of Scientific and Technical Information of China (English)
Zhang Hua
2005-01-01
In this paper we present for the first time the effects of Rayleigh scattering on the long distance propagation of ultraviolet (UV) light filament in air based on the stationary analysis. The simulation results show that the effects of Rayleigh scattering on the propagation of UV laser filaments may not be ignored. These influences are slightly dependent on the laser wavelength. We also compare the UV filament propagations at different input powers in the presence and the absence of the Rayleigh scattering and discuss the mechanisms of power loss and beam defocusing.In the absence of Rayleigh scattering, the filament propagation is determined by the oscillating behaviour of the beam size. In the presence of the scattering, the propagation lengths of filament are close to each other at different initial powers and determined by the Rayleigh scattering.
Quantifying light scattering with single-mode fiber -optic confocal microscopy
Directory of Open Access Journals (Sweden)
Haidekker Mark A
2009-11-01
Full Text Available Abstract Background Confocal microscopy has become an important option for examining tissues in vivo as a diagnostic tool and a quality control tool for tissue-engineered constructs. Collagen is one of the primary determinants of biomechanical stability. Since collagen is also the primary scattering element in skin and other soft tissues, we hypothesized that laser-optical imaging methods, particularly confocal scattered-light scanning, would allow us to quantify scattering intensity and determine collagen content in biological layers. Methods We built a fully automated confocal scattered-light scanner to examine how light scatters in Intralipid, a common tissue phantom, and three-dimensional collagen gels. Intralipid with 0.5%, 1.0%, 1.5%, and 2.0% concentration was filled between precisely spaced glass coverslips. Collagen gels at collagen concentrations from 0.30 mg/mL to 3.30 mg/mL were prepared, and all samples underwent A-mode scanning with multiple averaged scans. In Intralipid samples, light reflected from the upper fluid-glass interface was measured. In collagen gels, average scattering intensity inside the actual gel was measured. In both cases, intensity was correlated with concentration. Results By measuring light attenuation at interface reflections of various thicknesses using our device, we were able to determine that the scattering coefficient at 660 nm of Intralipid at increasing concentrations in water to be 39 cm-1 for each percent increase of Intralipid. We were also able to measure the amount of scattering of various concentrations of collagen in gels directly using backscattered light. The results show a highly linear relationship with an increase of 8.2 arbitrary units in backscattering intensity for every 1 mg increase of collagen within a 1 mL gel volume. Conclusion The confocal scattered-light scanner allows to accurately quantify scattering in Intralipid and collagen gels. Furthermore, a linear relationship between
Porsch, Bedrich; Welinder, Anette; Körner, Anna; Wittgren, Bengt
2005-03-18
Two different size-exclusion chromatography (SEC) systems, connected in-line either to a low-angle light scattering (LALS) or to a multiangle light scattering (MALS) detector, are employed for determination of molecular mass distributions (MMD) of poly(ethylene oxide) (PEO) samples having a weight average molecular mass up to eight millions. The detrimental effect of the presence of strongly scattering silica particles in the samples on the light scattering signal can be eliminated using a suitable sample dissolution procedure utilizing silica solubility in aqueous mobile phase. The selection of flow-rate and sample concentration have a large impact on the obtained results. Hydrodynamic retardation phenomena and nonlinearity effects are shown to introduce severe errors in the molecular mass distributions unless flow-rate and sample concentration are kept at sufficiently low levels. Self-compensating ability of the dual detection in flow-rate effects is shown to be the main advantage here. A good agreement between the results obtained using LALS and MALS detection is found provided that a carefully selected angular extrapolation procedure is used in the case of MALS data. Thus, using carefully selected experimental conditions, SEC with light-scattering (LS) and refractometric detection proved to be an efficient technique for MMD characterisation also of ultra-high molecular mass (UHM) PEO polymers.
Adhikari, S. K.
2016-09-01
We consider the statics and dynamics of a stable, mobile three-dimensional (3D) spatiotemporal light bullet in a cubic-quintic nonlinear medium with a focusing cubic nonlinearity above a critical value and any defocusing quintic nonlinearity. The 3D light bullet can propagate with a constant velocity in any direction. Stability of the light bullet under a small perturbation is established numerically. We consider frontal collision between two light bullets with different relative velocities. At large velocities the collision is elastic with the bullets emerge after collision with practically no distortion. At small velocities two bullets coalesce to form a bullet molecule. At a small range of intermediate velocities the localized bullets could form a single entity which expands indefinitely, leading to a destruction of the bullets after collision. The present study is based on an analytic Lagrange variational approximation and a full numerical solution of the 3D nonlinear Schrödinger equation.
Self-Organization of Light in Optical Media with Competing Nonlinearities.
Maucher, F; Pohl, T; Skupin, S; Krolikowski, W
2016-04-22
We study the propagation of light beams through optical media with competing nonlocal nonlinearities. We demonstrate that the nonlocality of competing focusing and defocusing nonlinearities gives rise to self-organization and stationary states with stable hexagonal intensity patterns, akin to transverse crystals of light filaments. Signatures of this long-range ordering are shown to be observable in the propagation of light in optical waveguides and even in free space. We consider a specific form of the nonlinear response that arises in atomic vapor upon proper light coupling. Yet, the general phenomenon of self-organization is a generic consequence of competing nonlocal nonlinearities, and may, hence, also be observed in other settings.
Bartolini, R.
2016-01-01
This paper introduces the most recent achievements in the control of nonlinear dynamics in electron synchrotron light sources, with special attention to diffraction limited storage rings. Guidelines for the design and optimization of the magnetic lattice are reviewed and discussed.
Impact of polishing on the light scattering at aerogel surface
Energy Technology Data Exchange (ETDEWEB)
Barnyakov, A.Yu. [Budker Institute of Nuclear Physics SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Barnyakov, M.Yu. [Budker Institute of Nuclear Physics SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Novosibirsk State Technical University, Novosibirsk (Russian Federation); Bobrovnikov, V.S.; Buzykaev, A.R. [Budker Institute of Nuclear Physics SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Danilyuk, A.F. [Novosibirsk State University, Novosibirsk (Russian Federation); Boreskov Institute of Catalysis SB RAS, Novosibirsk (Russian Federation); Katcin, A.A. [Budker Institute of Nuclear Physics SB RAS, Novosibirsk (Russian Federation); Novosibirsk State Technical University, Novosibirsk (Russian Federation); Kononov, S.A. [Budker Institute of Nuclear Physics SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Kirilenko, P.S. [Novosibirsk State University, Novosibirsk (Russian Federation); Kravchenko, E.A., E-mail: E.A.Kravchenko@inp.nsk.su [Budker Institute of Nuclear Physics SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Kuyanov, I.A. [Budker Institute of Nuclear Physics SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Onuchin, A.P.; Ovtin, I.V. [Budker Institute of Nuclear Physics SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Novosibirsk State Technical University, Novosibirsk (Russian Federation); Predein, A.Yu.; Protsenko, R.S. [Boreskov Institute of Catalysis SB RAS, Novosibirsk (Russian Federation)
2016-07-11
Particle identification power of modern aerogel RICH detectors strongly depends on optical quality of radiators. It was shown that wavelength dependence of aerogel tile transparency after polishing cannot be described by the standard Hunt formula. The Hunt formula has been modified to describe scattering in a thin layer of silica dust on the surface of aerogel tile. Several procedures of polishing of aerogel tile have been tested. The best result has been achieved while using natural silk tissue. The resulting block has optical smooth surfaces. The measured decrease of aerogel transparency due to surface scattering is about few percent. This result could be used for production of radiators for the Focusing Aerogel RICH detectors.
Temporal Quantum Correlations in Inelastic Light Scattering from Water
Kasperczyk, Mark; de Aguiar Júnior, Filomeno S.; Rabelo, Cassiano; Saraiva, Andre; Santos, Marcelo F.; Novotny, Lukas; Jorio, Ado
2016-12-01
Water is one of the most prevalent chemicals on our planet, an integral part of both our environment and our existence as a species. Yet it is also rich in anomalous behaviors. Here we reveal that water is a novel—yet ubiquitous—source for quantum correlated photon pairs at ambient conditions. The photon pairs are produced through Raman scattering, and the correlations arise from the shared quantum of a vibrational mode between the Stokes and anti-Stokes scattering events. We confirm the nonclassical nature of the produced photon pairs by showing that the cross-correlation and autocorrelations of the signals violate a Cauchy-Schwarz inequality by over 5 orders of magnitude. The unprecedented degree of violating the inequality in pure water, as well as the well-defined polarization properties of the photon pairs, points to its usefulness in quantum information.
Resonant chirality in light scattered from magnetodielectric particles
Nieto-Vesperinas, Manuel
2016-01-01
We show that the total heliciity of the field scattered by a magnetodielectric particle, bi-isotropic or not, is enhanced not only because of the resonant polarizabilities, but also due to the interference between the left and right circularly polarized components of the incident wave, which in absence of incident helicity does not necessarily require the particle to be chiral. This latter effect goes beyond standard dichroism and may be considered a generalization of this phenomenon.
Maximizing the information transfer in a quantum-limited light-scattering system
DEFF Research Database (Denmark)
Lading, Lars; Jørgensen, Thomas Martini
1990-01-01
A quantum-limited light-scattering system is considered. The spatial configuration that maximizes a given figure of merit is investigated, assuming that the emitted light has Poisson photon statistics. A specific system for measuring the velocity of a small particle is considered as an example...
Observation of spatial quantum correlations induced by multiple scattering of nonclassical light
DEFF Research Database (Denmark)
Smolka, Stephan; Huck, Alexander; Andersen, Ulrik Lund;
2009-01-01
We present the experimental realization of spatial quantum correlations of photons that are induced by multiple scattering of squeezed light. The quantum correlation relates photons propagating along two different light paths through the random medium and is infinite in range. Both positive...
Institute of Scientific and Technical Information of China (English)
LI Wei; GAO Feng; TANG Bai-Quan; Christian Pruner; ZHANG Xin-Zheng; SHI Yan-Li; XU Jing-Jun; QIAO Hai-Jun; WU Qiang; Romano A. Rupp; LOU Ci-Bo; WANG Zhen-Hua
2008-01-01
@@ Light amplification due to two-beam coupling is realized in doped polymethyl methacrylate (PMMA) glasses. A coupling gain as large as 14 cm-1 is obtained. The dynamic behaviour of absorption and light-induced scattering due to the process of photopolymerization are also studied. The results show that the amplification and its dynamic process enable possible applications of PMMA in optical devices.
Preston, Thomas C; Reid, Jonathan P
2015-06-01
The angular scattering of light from a homogeneous spherical particle in a zeroth-order Bessel beam is calculated using a generalized Lorenz-Mie theory. We investigate the dependence of the angular scattering on the semi-apex angle of the Bessel beam and discuss the major features of the resulting scattering plots. We also compare Bessel beam scattering to plane wave scattering and provide criterion for when the difference between the two cases can be considered negligible. Finally, we discuss a method for characterizing spherical particles using angular light scattering. This work is useful to researchers who are interested in characterizing particles trapped in optical beams using angular dependent light scattering measurements.
Matsuda, Nobuyuki; Kato, Takumi; Harada, Ken-Ichi; Takesue, Hiroki; Kuramochi, Eiichi; Taniyama, Hideaki; Notomi, Masaya
2011-10-10
We demonstrate highly enhanced optical nonlinearity in a coupled-resonator optical waveguide (CROW) in a four-wave mixing experiment. Using a CROW consisting of 200 coupled resonators based on width-modulated photonic crystal nanocavities in a line defect, we obtained an effective nonlinear constant exceeding 10,000 /W/m, thanks to slow light propagation combined with a strong spatial confinement of light achieved by the wavelength-sized cavities.
Wang, Geng; Su, Zhenpeng; Zheng, Huinan; Wang, Yuming; Zhang, Min; Wang, Shui
2017-02-01
Cyclotron resonant scattering by electromagnetic ion cyclotron (EMIC) waves has been considered to be responsible for the rapid loss of radiation belt high-energy electrons. For parallel-propagating EMIC waves, the nonlinear character of cyclotron resonance has been revealed in recent studies. Here we present the first study on the nonlinear fundamental and harmonic cyclotron resonant scattering of radiation belt ultrarelativistic electrons by oblique EMIC waves on the basis of test particle simulations. Higher wave obliquity produces stronger nonlinearity of harmonic resonances but weaker nonlinearity of fundamental resonance. Compared to the quasi-linear prediction, these nonlinear resonances yield a more rapid loss of electrons over a wider pitch angle range. In the quasi-linear regime, the ultrarelativistic electrons are lost in the equatorial pitch angle range αeq87.5° at ψ = 20° and 40°. At the resonant pitch angles αeq<75°, the difference between quasi-linear and nonlinear loss timescales tends to decrease with the wave normal angle increasing. At ψ = 0° and 20°, the nonlinear electron loss timescale is 10% shorter than the quasi-linear prediction; at ψ = 40°, the difference in loss timescales is reduced to <5%.
Egel, Amos; Gomard, Guillaume; Kettlitz, Siegfried W.; Lemmer, Uli
2017-02-01
We present a numerical strategy for the accurate simulation of light extraction from organic light emitting diodes (OLEDs) comprising an internal nano-particle based scattering layer. On the one hand, the light emission and propagation through the OLED thin film system (including the scattering layer) is treated by means of rigorous wave optics calculations using the T-matrix formalism. On the other hand, the propagation through the substrate is modeled in a ray optics approach. The results from the wave optics calculations enter in terms of the initial substrate radiation pattern and the bidirectional reflectivity distribution of the OLED stack with scattering layer. In order to correct for the truncation error due to a finite number of particles in the simulations, we extrapolate the results to infinitely extended scattering layers. As an application example, we estimate the optimal particle filling fraction for an internal scattering layer in a realistic OLED geometry. The presented treatment is designed to emerge from electromagnetic theory with as few additional assumptions as possible. It could thus serve as a baseline to validate faster but approximate simulation approaches.
Directory of Open Access Journals (Sweden)
Y. Sakai
2017-06-01
Full Text Available Inverse Compton scattering (ICS is a unique mechanism for producing fast pulses—picosecond and below—of bright photons, ranging from x to γ rays. These nominally narrow spectral bandwidth electromagnetic radiation pulses are efficiently produced in the interaction between intense, well-focused electron and laser beams. The spectral characteristics of such sources are affected by many experimental parameters, with intense laser effects often dominant. A laser field capable of inducing relativistic oscillatory motion may give rise to harmonic generation and, importantly for the present work, nonlinear redshifting, both of which dilute the spectral brightness of the radiation. As the applications enabled by this source often depend sensitively on its spectra, it is critical to resolve the details of the wavelength and angular distribution obtained from ICS collisions. With this motivation, we present an experimental study that greatly improves on previous spectral measurement methods based on x-ray K-edge filters, by implementing a multilayer bent-crystal x-ray spectrometer. In tandem with a collimating slit, this method reveals a projection of the double differential angular-wavelength spectrum of the ICS radiation in a single shot. The measurements enabled by this diagnostic illustrate the combined off-axis and nonlinear-field-induced redshifting in the ICS emission process. The spectra obtained illustrate in detail the strength of the normalized laser vector potential, and provide a nondestructive measure of the temporal and spatial electron-laser beam overlap.
Sakai, Y.; Gadjev, I.; Hoang, P.; Majernik, N.; Nause, A.; Fukasawa, A.; Williams, O.; Fedurin, M.; Malone, B.; Swinson, C.; Kusche, K.; Polyanskiy, M.; Babzien, M.; Montemagno, M.; Zhong, Z.; Siddons, P.; Pogorelsky, I.; Yakimenko, V.; Kumita, T.; Kamiya, Y.; Rosenzweig, J. B.
2017-06-01
Inverse Compton scattering (ICS) is a unique mechanism for producing fast pulses—picosecond and below—of bright photons, ranging from x to γ rays. These nominally narrow spectral bandwidth electromagnetic radiation pulses are efficiently produced in the interaction between intense, well-focused electron and laser beams. The spectral characteristics of such sources are affected by many experimental parameters, with intense laser effects often dominant. A laser field capable of inducing relativistic oscillatory motion may give rise to harmonic generation and, importantly for the present work, nonlinear redshifting, both of which dilute the spectral brightness of the radiation. As the applications enabled by this source often depend sensitively on its spectra, it is critical to resolve the details of the wavelength and angular distribution obtained from ICS collisions. With this motivation, we present an experimental study that greatly improves on previous spectral measurement methods based on x-ray K -edge filters, by implementing a multilayer bent-crystal x-ray spectrometer. In tandem with a collimating slit, this method reveals a projection of the double differential angular-wavelength spectrum of the ICS radiation in a single shot. The measurements enabled by this diagnostic illustrate the combined off-axis and nonlinear-field-induced redshifting in the ICS emission process. The spectra obtained illustrate in detail the strength of the normalized laser vector potential, and provide a nondestructive measure of the temporal and spatial electron-laser beam overlap.
Skeletal light-scattering accelerates bleaching response in reef-building corals.
Swain, Timothy D; DuBois, Emily; Gomes, Andrew; Stoyneva, Valentina P; Radosevich, Andrew J; Henss, Jillian; Wagner, Michelle E; Derbas, Justin; Grooms, Hannah W; Velazquez, Elizabeth M; Traub, Joshua; Kennedy, Brian J; Grigorescu, Arabela A; Westneat, Mark W; Sanborn, Kevin; Levine, Shoshana; Schick, Mark; Parsons, George; Biggs, Brendan C; Rogers, Jeremy D; Backman, Vadim; Marcelino, Luisa A
2016-03-21
At the forefront of ecosystems adversely affected by climate change, coral reefs are sensitive to anomalously high temperatures which disassociate (bleaching) photosynthetic symbionts (Symbiodinium) from coral hosts and cause increasingly frequent and severe mass mortality events. Susceptibility to bleaching and mortality is variable among corals, and is determined by unknown proportions of environmental history and the synergy of Symbiodinium- and coral-specific properties. Symbiodinium live within host tissues overlaying the coral skeleton, which increases light availability through multiple light-scattering, forming one of the most efficient biological collectors of solar radiation. Light-transport in the upper ~200 μm layer of corals skeletons (measured as 'microscopic' reduced-scattering coefficient, μ'(S,m)), has been identified as a determinant of excess light increase during bleaching and is therefore a potential determinant of the differential rate and severity of bleaching response among coral species. Here we experimentally demonstrate (in ten coral species) that, under thermal stress alone or combined thermal and light stress, low-μ'(S,m) corals bleach at higher rate and severity than high-μ'(S,m) corals and the Symbiodinium associated with low-μ'(S,m) corals experience twice the decrease in photochemical efficiency. We further modelled the light absorbed by Symbiodinium due to skeletal-scattering and show that the estimated skeleton-dependent light absorbed by Symbiodinium (per unit of photosynthetic pigment) and the temporal rate of increase in absorbed light during bleaching are several fold higher in low-μ'(S,m) corals. While symbionts associated with low-[Formula: see text] corals receive less total light from the skeleton, they experience a higher rate of light increase once bleaching is initiated and absorbing bodies are lost; further precipitating the bleaching response. Because microscopic skeletal light-scattering is a robust predictor
Enhancing Localized Evaporation through Separated Light Absorbing Centers and Scattering Centers.
Zhao, Dengwu; Duan, Haoze; Yu, Shengtao; Zhang, Yao; He, Jiaqing; Quan, Xiaojun; Tao, Peng; Shang, Wen; Wu, Jianbo; Song, Chengyi; Deng, Tao
2015-11-26
This report investigates the enhancement of localized evaporation via separated light absorbing particles (plasmonic absorbers) and scattering particles (polystyrene nanoparticles). Evaporation has been considered as one of the most important phase-change processes in modern industries. To improve the efficiency of evaporation, one of the most feasible methods is to localize heat at the top water layer rather than heating the bulk water. In this work, the mixture of purely light absorptive plasmonic nanostructures such as gold nanoparticles and purely scattering particles (polystyrene nanoparticles) are employed to confine the incident light at the top of the solution and convert light to heat. Different concentrations of both the light absorbing centers and the light scattering centers were evaluated and the evaporation performance can be largely enhanced with the balance between absorbing centers and scattering centers. The findings in this study not only provide a new way to improve evaporation efficiency in plasmonic particle-based solution, but also shed lights on the design of new solar-driven localized evaporation systems.
Non-Linear Compton Scattering in a Strong Rotating Electric Field
Raicher, Erez; Zigler, Arie
2016-01-01
The non-linear Compton scattering rate in a rotating electric field is explicitly calculated for the first time. For this purpose, a novel solution to the Klein-Gordon equation in the presence of a rotating electric field is applied. An analytical expression for the emission rate is obtained, as well as a simplified approximation adequate for emplementation in kinetic codes. The spectrum is numerically calculated for nowadays optical and X-ray laser parameters. The results are compared to the standard Volkov-Ritus rate for a particle in a plane wave, which is commonly assumed to be valid for a rotating electric field under certain conditions. Subsequent deviations between the two models, both in the radiated power and the spectral shape, are demonstrated. First, the typical number of photons participating in the scattering process is much smaller compared to the Volkov-Ritus rate, resulting in up to an order of magnitude lower emitted power. Furthermore, our model predicts a discrete harmonics spectrum for el...
Role of orbital filling on nonlinear ionic Raman scattering in perovskite titanates
Gu, Mingqiang; Rondinelli, James M.
2017-01-01
The linear and nonlinear phononic interactions between an optically excited infrared (IR) or hyper-Raman mode and a driven Raman mode are computed for the d0 (CaTiO3) and d1 (LaTiO3) titanates within a first-principles density functional framework. We calculate the potential energy surface expanded in terms of the Ag or B1 g mode amplitudes coupled to the Au or the B3 u mode and determine the coupling coefficients for these multimode interactions. We find that the linear-quadratic coupling dominates the anharmonicities over the quadratic-quadratic interaction in the perovskite titanates. The IR and Raman modes both modify the electronic structure with the former being more significant but occurring on a different time scale; furthermore, the coupled-mode interactions lead to sizable perturbations to the valence bandwidth (˜100 meV ) and band gap (˜50 meV). By comparing the coupling coefficients of undoped CaTiO3 and LaTiO3 to those for electron-doped (CaTiO3) and hole-doped (LaTiO3) titanates, we isolate the role of orbital filling in the nonlinear coupling process. We find that with increasing occupancy of the d manifold, the linear-quadratic interaction decreases by approximately 30% with minor changes induced by the cation chemistry (that mainly affect the phonon mode frequencies) or by electron correlation. We identify the importance of the Ti-O bond stiffness, which depends on the orbital filling, in governing the lattice anharmonicitiy. This microscopic understanding can be used to increase the nonlinear coupling coefficient to facilitate more facile access of nonequilibrium structures and properties through ionic Raman scattering processes.
Simulations of the Light Scattering Properties of Metal/Oxide Core/Shell Nanospheres
Directory of Open Access Journals (Sweden)
F. Ruffino
2014-01-01
Full Text Available Given the importance of the optical properties of metal/dielectric core/shell nanoparticles, in this work we focus our attention on the light scattering properties, within the Mie framework, of some specific categories of these noteworthy nanostructures. In particular, we report theoretical results of angle-dependent light scattering intensity and scattering efficiency for Ag/Ag2O, Al/Al2O2, Cu/Cu2O, Pd/PdO, and Ti/TiO2 core/shell nanoparticles as a function of the core radius/shell thickness ratio and on a relative comparison. The results highlight the light scattering characteristics of these systems as a function of the radius/shell thickness ratio, helping in the choice of the more suitable materials and sizes for specific applications (i.e., dynamic light scattering for biological and molecular recognition, increasing light trapping in thin-film silicon, organic solar cells for achieving a higher photocurrent.
Asahi, Ippei; Ninomiya, Hideki
An experimental study to visualize and measure the concentration distribution of hydrogen gas flow using the Raman scattering was performed. A Nd:YAG laser of wavelength at 355 nm was used, and the beam pattern was transformed into a rectangle and a sheet beam was formed. The Raman scattered light was observed at a right angle with respect to the laser beam axis using a gated ICCD camera and an interference filter. Shadowgraph images were obtained at the same condition. The Raman scattering light image from atmospheric nitrogen was first acquired and the function of Raman scattering light acquisition and the background light suppression was confirmed. Next, images of the Raman scattering light image and shadowgraph of hydrogen gas discharged from a nozzle into the atmosphere were acquired. The two obtained Raman images were compared and the spatial concentration distribution of the flow of the hydrogen gas at different flow rates was calculated. This method is effective for visualizing the gas flow and measuring the concentration distribution of the Raman active molecules, such as hydrogen gas.
Optical fibre probes in the measurement of scattered light: Application for sensing turbidity
Indian Academy of Sciences (India)
M R Sheno
2014-01-01
Optical fibre probes or optrodes often form the heart of multimode fibre-based measurements and sensors. An optrode usually comprises a bundle of multimode fibres, out of which one or more fibres are used for irradiating the sample, and the remaining fibres are used to collect the light reflected/scattered/fluoresced from the sample containing the measurand(s). The so-collected light carries the characteristic signature of the measurand. Here we present our work on the design and realization of optrodes for the measurement of scattered light from liquid samples. Optical properties of a solution are usually characterized by the parameters absorption coefficient $_a$, scattering coefficient $_s$, and anisotropy factor . We have developed a simple method to determine $_a$, $_s$, and , of a turbid medium, and a Monte–Carlo model was used to simulate the light scattering from the turbid medium. As an application, we describe the development of a turbidity sensor that has been designed and realized by employing an optrode in conjunction with a concave mirror. The estimation of turbidity is done on the basis of total interaction, by considering scattering and absorption of light from the sample solution. Details of the experiments and results are presented here.
Institute of Scientific and Technical Information of China (English)
NIU Jia-Sheng; MA Ben-Kun
2003-01-01
In this paper, we theoretically discuss the soliton properties of light pulse transportation on the surface of an ionic crystal having strong nonlinear interactions between ions of unit cells. We analyze in detail the dark solitons when the nonlinear coefficient g is positive and negative, respectively. It is found that whether the nonlinear coefficient g is positive or negative, the dark solitons can be formed over the whole dispersion relation area of surface polaritons considering nonlinear effects. Attention should be paid to the fact that around ωTO, the light pulse can form advanced dark solitons, and there is a switching area from advanced dark soliton to retarded dark soliton near ωTO. We also discuss the effects of higher nonlinear dispersion on the solitons.
Bragg-Scattering Four-Wave Mixing in Nonlinear Fibers with Intracavity Frequency-Shifted Laser Pumps
Directory of Open Access Journals (Sweden)
Katarzyna Krupa
2012-01-01
Full Text Available We experimentally study four-wave mixing in highly nonlinear fibers using two independent and partially coherent laser pumps and a third coherent signal. We focus our attention on the Bragg-scattering frequency conversion. The two pumps were obtained by amplifying two Intracavity frequency-shifted feedback lasers working in a continuous wave regime.
The light filament as a new nonlinear polarization state
Kovachev, Lubomir M
2015-01-01
We present an analytical approach to the theory of nonlinear propagation in gases of femtosecond optical pulses with broad-band spectrum . The vector character of the nonlinear third-order polarization of the electrical field in air is investigated in details. A new polarization state is presented by using left-hand and right-hand circular components of the electrical field . The corresponding system of vector amplitude equations is derived in the rotating basis. We found that this system of nonlinear equations has $3D+1$ vector soliton solutions with Lorentz shape. The solution presents a relatively stable propagation and rotation with GHz frequency of the vector of the electrical field in a plane orthogonal to the direction of propagation. The evolution of the intensity profile demonstrates a weak self-compression and a week spherical wave in the first milliseconds of propagation.
Brustlein, Sophie; Ferrand, Patrick; Walther, Nico; Brasselet, Sophie; Billaudeau, Cyrille; Marguet, Didier; Rigneault, Hervé
2011-02-01
We present the assets and constraints of using optical parametric oscillators (OPOs) to perform point scanning nonlinear microscopy and spectroscopy with special emphasis on coherent Raman spectroscopy. The difterent possible configurations starting with one OPO and two OPOs are described in detail and with comments that are intended to be practically useful for the user. Explicit examples on test samples such as nonlinear organic crystal, polystyrene beads, and fresh mouse tissues are given. Special emphasis is given to background-free coherent Raman anti-Stokes scattering (CARS) imaging, including CARS hyperspectral imaging in a fully automated mode with commercial OPOs.
Controlling light in scattering media noninvasively using the photo-acoustic transmission-matrix
Chaigne, T; Boccara, A C; Fink, M; Bossy, E; Gigan, S
2013-01-01
Optical wavefront-shaping has emerged as a powerful tool to manipulate light in strongly scattering media. It enables diffraction-limited focusing and imaging at depths where conventional microscopy techniques fail. However, while most wavefront-shaping works to-date exploited direct access to the target or implanted probes, the challenge is to apply it non-invasively inside complex samples. Ultrasonic-tagging techniques have been recently demonstrated but these require a sequential point-by- point acquisition, a major drawback for imaging applications. Here, we introduce a novel approach to non-invasively measure the optical transmission-matrix inside a scattering medium, exploiting the photo-acoustic effect. Our approach allows for the first time to simultaneously discriminate, localize, and selectively focus light on multiple targets inside a scattering sample, as well as to recover and exploit the scattering medium properties. Combining the powerful approach of the transmission-matrix with the advantages ...
Modal theory of slow light enhanced third-order nonlinear effects in photonic crystal waveguides.
Chen, Tao; Sun, Junqiang; Li, Linsen
2012-08-27
In this paper, we derive the couple-mode equations for third-order nonlinear effects in photonic crystal waveguides by employing the modal theory. These nonlinear interactions include self-phase modulation, cross-phase modulation and degenerate four-wave mixing. The equations similar to that in nonlinear fiber optics could be expanded and applied for third-order nonlinear processes in other periodic waveguides. Based on the equations, we systematically analyze the group-velocity dispersion, optical propagation loss, effective interaction area, slow light enhanced factor and phase mismatch for a slow light engineered silicon photonic crystal waveguide. Considering the two-photon and free-carrier absorptions, the wavelength conversion efficiencies in two low-dispersion regions are numerically simulated by utilizing finite difference method. Finally, we investigate the influence of slow light enhanced multiple four-wave-mixing process on the conversion efficiency.
Shinkawa, Mizuki; Ishikura, Norihiro; Hama, Yosuke; Suzuki, Keijiro; Baba, Toshihiko
2011-10-24
We have studied low-dispersion slow light and its nonlinear enhancement in photonic crystal waveguides. In this work, we fabricated the waveguides using Si CMOS-compatible process. It enables us to integrate spotsize converters, which greatly simplifies the optical coupling from fibers as well as demonstration of the nonlinear enhancement. Two-photon absorption, self-phase modulation and four-wave mixing were observed clearly for picosecond pulses in a 200-μm-long device. In comparison with Si wire waveguides, a 60-120 fold higher nonlinearity was evaluated for a group index of 51. Unique intensity response also occurred due to the specific transmission spectrum and enhanced nonlinearities. Such slow light may add various functionalities in Si photonics, while loss reduction is desired for ensuring the advantage of slow light.
Scattering of light halo nuclei on heavy target at energies around the Coulomb barrier
Directory of Open Access Journals (Sweden)
Tengblad O.
2014-03-01
Full Text Available We report here on experiments performed at TRIUMF to study the scattering of the light halo nuclei 11Li on lead at energies below and around the Coulomb barrier. The the elastic and break-up differential cross section are interpreted in the framework of Continuum-Discretized Coupled-Channel calculations. The departure from Rutherford scattering at energies below the barrier is well beyond the behavior of normal nuclei.
Williams, L. M.; Cummins, H. Z.; Ladeira, L. O.; Mesquita, O. N.
1992-03-01
We have investigated the phenomenon of intense dynamic light scattering at the nonequilibrium crystal-melt interface in succinonitrile and naphthalene, in order to resolve the ongoing controversy over its origin. Of the several models that have been proposed to explain this phenomenon, the microbubble model of H. Z. Cummins et al. [Solid State Commun. 60, 857 (1986)] and the mesophase model proposed by J. Bilgram and co-workers [P. Boni, J. H. Bilgram, and W. Kanzig, Phys. Rev. A 28, 2953 (1983)] are the only two still considered to be consistent with most of the experimental observations. In these experiments the angular dependence of the scattered light was investigated. In the mesophase model the angular dependence of the scattered light is described by the Ornstein-Zernike form I(q)=I0(1+q2ξ2)-1, whereas light scattered by bubbles can be modeled by the Mie scattering theory. The data for both materials were found to be incompatible with the Ornstein-Zernike form, but could be reasonably well fit by the Mie theory. The behavior of the onset of scattering was also investigated, and it was found that the product R0t0v2g was a constant, where R0 is the onset radius, t0 the onset time, and vg the crystal growth velocity. This result is consistent with the analysis of Mesquita et al. [Phys. Rev. B 38, 1550 (1988)], in which the onset of the scattering was modeled by considering the rate of buildup of dissolved gas at the advancing crystal-melt interface. The time taken for the disappearance of the scattering after growth was terminated was also investigated. Lastly, the gases dissolved in our samples of succinonitrile were identified by mass spectroscopy and found to have a composition similar to air.
Scattering of light halo nuclei on heavy target at energies around the Coulomb barrier
Tengblad O.; Borge M.J.G.; Cubero M.; Nacher E.; Pesudo V.; Perea A.; Gomez-Camacho J.; Moro A. M.; Fernandez-Garcia J.P.; Alvarez M.A.G.; Rodriguez-Gallardo M.; Lay J. A.; Martel I.; Acosta L.; Sanchez-Benitez A.M.
2014-01-01
INPC 2013 – International Nuclear Physics Conference We report here on experiments performed at TRIUMF to study the scattering of the light halo nuclei 11Li on lead at energies below and around the Coulomb barrier. The the elastic and break-up differential cross section are interpreted in the framework of Continuum-Discretized Coupled-Channel calculations. The departure from Rutherford scattering at energies below the barrier is well beyond the behavior of normal nuclei Consejo Interins...
Characterization of the angular memory effect of scattered light in biological tissues
Schott, Sam; Léger, Jean-Francois; Bourdieu, Laurent; Gigan, Sylvain
2015-01-01
High resolution optical microscopy is essential in neuroscience but suffers from scattering in biological tissues. It therefore grants access to superficial layers only. Recently developed techniques use scattered photons for imaging by exploiting angular correlations in transmitted light and could potentially increase imaging depths. But those correlations (`angular memory effect') are of very short range and, in theory, only present behind and not inside scattering media. From measurements on neural tissues and complementary simulations, we find that strong forward scattering in biological tissues can enhance the memory effect range (and thus the possible field-of-view) by more than an order of magnitude compared to isotropic scattering for $\\sim$1\\,mm thick tissue layers.
Characterization of the angular memory effect of scattered light in biological tissues
Schott, Sam; Bertolotti, Jacopo; Léger, Jean-Francois; Bourdieu, Laurent; Gigan, Sylvain
2015-05-01
High resolution optical microscopy is essential in neuroscience but suffers from scattering in biological tissues. It therefore grants access to superficial layers only. Recently developed techniques use scattered photons for imaging by exploiting angular correlations in transmitted light and could potentially increase imaging depths. But those correlations (`angular memory effect') are of very short range and, in theory, only present behind and not inside scattering media. From measurements on neural tissues and complementary simulations, we find that strong forward scattering in biological tissues can enhance the memory effect range (and thus the possible field-of-view) by more than an order of magnitude compared to isotropic scattering for $\\sim$1\\,mm thick tissue layers.
Characterization of the angular memory effect of scattered light in biological tissues.
Schott, Sam; Bertolotti, Jacopo; Léger, Jean-Francois; Bourdieu, Laurent; Gigan, Sylvain
2015-05-18
High resolution optical microscopy is essential in neuroscience but suffers from scattering in biological tissues and therefore grants access to superficial brain layers only. Recently developed techniques use scattered photons for imaging by exploiting angular correlations in transmitted light and could potentially increase imaging depths. But those correlations ('angular memory effect') are of a very short range and should theoretically be only present behind and not inside scattering media. From measurements on neural tissues and complementary simulations, we find that strong forward scattering in biological tissues can enhance the memory effect range and thus the possible field-of-view by more than an order of magnitude compared to isotropic scattering for ∼1 mm thick tissue layers.
Focusing light inside dynamic scattering media with millisecond digital optical phase conjugation.
Liu, Yan; Ma, Cheng; Shen, Yuecheng; Shi, Junhui; Wang, Lihong V
2017-02-01
Wavefront shaping based on digital optical phase conjugation (DOPC) focuses light through or inside scattering media, but the low speed of DOPC prevents it from being applied to thick, living biological tissue. Although a fast DOPC approach was recently developed, the reported single-shot wavefront measurement method does not work when the goal is to focus light inside, instead of through, highly scattering media. Here, using a ferroelectric liquid crystal based spatial light modulator, we develop a simpler but faster DOPC system that focuses light not only through, but also inside scattering media. By controlling 2.6 × 10(5) optical degrees of freedom, our system focused light through 3 mm thick moving chicken tissue, with a system latency of 3.0 ms. Using ultrasound-guided DOPC, along with a binary wavefront measurement method, our system focused light inside a scattering medium comprising moving tissue with a latency of 6.0 ms, which is one to two orders of magnitude shorter than those of previous digital wavefront shaping systems. Since the demonstrated speed approaches tissue decorrelation rates, this work is an important step toward in vivo deep-tissue non-invasive optical imaging, manipulation, and therapy.
A new dump system design for stray light reduction of Thomson scattering diagnostic system on EAST
Xiao, Shumei; Zang, Qing; Han, Xiaofeng; Wang, Tengfei; Yu, Jin; Zhao, Junyu
2016-07-01
Thomson scattering (TS) diagnostic is an important diagnostic for measuring electron temperature and density during plasma discharge. However, the measurement of Thomson scattering signal is disturbed by the stray light easily. The stray light sources in the Experimental Advanced Superconducting Tokamak (EAST) TS diagnostic system were analyzed by a simulation model of the diagnostic system, and simulation results show that the dump system is the primary stray light source. Based on the optics theory and the simulation analysis, a novel dump system including an improved beam trap was proposed and installed. The measurement results indicate that the new dump system can reduce more than 60% of the stray light for the diagnostic system, and the influence of stray light on the error of measured density decreases.
Institute of Scientific and Technical Information of China (English)
Marimuthu PAULVANNA NAYAKI; Arunachalam P. KABILAN
2009-01-01
A novel light scattering technique for mapping metal surface corrosion is presented and its results on copper exposed to atmosphere are reported. The front end of the instrument is made up of a sensor module comprising a thin beam light emitting diode (LED) illuminating a small spot on the metal surface, and a matched pair of photodetectors, one for capturing the reflected light and the other for sampling the scattered light. The analog photocurrent signals are digitized and processed online by a personal computer (PC) to determine the corrosion factor defined in terms of the two current values. By scanning the sample surface using the light beam and by computing the corrosion factor values simultaneously, a three dimensional graph and a two dimensional contour map are generated in the PC using Matlab tools. The values of the corrosion factor measured in different durations of exposure to atmosphere, which obey a bilogarithmic law, testify to the validity of our mathematical model.
A new dump system design for stray light reduction of Thomson scattering diagnostic system on EAST.
Xiao, Shumei; Zang, Qing; Han, Xiaofeng; Wang, Tengfei; Yu, Jin; Zhao, Junyu
2016-07-01
Thomson scattering (TS) diagnostic is an important diagnostic for measuring electron temperature and density during plasma discharge. However, the measurement of Thomson scattering signal is disturbed by the stray light easily. The stray light sources in the Experimental Advanced Superconducting Tokamak (EAST) TS diagnostic system were analyzed by a simulation model of the diagnostic system, and simulation results show that the dump system is the primary stray light source. Based on the optics theory and the simulation analysis, a novel dump system including an improved beam trap was proposed and installed. The measurement results indicate that the new dump system can reduce more than 60% of the stray light for the diagnostic system, and the influence of stray light on the error of measured density decreases.
Self-guiding light in layered nonlinear media
DEFF Research Database (Denmark)
Bergé, L.; Mezentsev, V. K.; Juul Rasmussen, Jens;
2000-01-01
We study the propagation of intense optical beams in layered Kerr media. With appropriate shapes, beams with a power close to the self-focusing threshold are shown to propagate over long distances as quasistationary waveguides in cubic media supporting a periodic nonlinear refractive index. (C...
Inelastic light scattering by low-lying excitations of electrons in low-dimensional semiconductors
Energy Technology Data Exchange (ETDEWEB)
Pellegrini, V. [NEST CNR-INFM and Scuola Normale Superiore, Pisa (Italy); Pinczuk, A. [Department of Physics, Department of Applied Physics and Applied Mathematics, Columbia University, New York, New York 10027 (United States); Bell Laboratories, Lucent Technologies, Murray Hill, New Jersey (United States)
2006-11-15
The low-dimensional electron systems that reside in artificial semiconductor heterostructures of great perfection are a contemporary materials base for explorations of collective phenomena. Studies of low-lying elementary excitations by inelastic light scattering offer insights on properties such energetics, interactions and spin magnetization. We review here recent light scattering results obtained from two-dimensional (2D) quantum fluids in semiconductor heterostructures under extreme conditions of low temperature and large magnetic field, where the quantum Hall phases are archetypes of novel behaviors. We also consider recent light scattering experiments that have probed the excitation spectra of few-electron states in semiconductor quantum dots. (copyright 2006 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)
Applications of Optical Sensors to the Detection of Light Scattered from Gelling Systems
Bulone, Donatella; Manno, Mauro; San Biagio, Pier Luigi; Martorana, Vincenzo
Visible light, scattered within an angle of few degrees, (Small Angle Light Scattering, SALS) yields information on the spatial correlations and dynamical properties on the scale of the micrometers. In this way a quick and non-invasive characterization of a variety of samples is feasible. Lately the SALS instruments have been built around multielement optical sensors (CCD, CMOS), allowing the simultaneous measurement of the complete structure factor even during fast kinetics. An assessment of some sensor matrices of different technology will be presented. The omolecular assemblies produced by polysaccharides or proteins can be functional or dysfunctional, their properties being either desirable or detrimental. Anyhow, their morphology often depends, in a very delicate way, on the presence of cosolutes, on the thermal history, on the biopolymer concentration etc. We present some applications of low angle dynamic and static light scattering to the study of gelling systems (agarose, pectin, insulin).
Development of 3D control of a tiny dew droplet by scattered laser light
Matsumoto, Shigeaki
2009-06-01
In order to study dropwise condensation on a metal plate, the method for controlling a tiny dew droplet deposited on a copper plate has been developed by using scattered laser light. The method employed the proportional control combined with shifting movement by an integrator to control the intensity of the scattered laser light constantly. Also, the control simulation of the method has been developed to confirm the usefulness of the method and the simulated three-dimensional shape of controlled dew droplet was obtained with the control action. A tiny thin dew droplet, of which the diameter was of handreds micrometers and the mass was about 10-7 g, was controlled in the atmosphere at room temperature for 60 minutes at the preset level of the intensity of scattered laser light and the three-dimensional shape of the controlled dew droplet was shown from the interference fringes.
Determination of liquid-liquid critical point composition using 90∘ laser light scattering
Williamson, J. Charles; Brown, Allison M.; Helvie, Elise N.; Dean, Kevin M.
2016-04-01
Despite over a century of characterization efforts, liquid-liquid critical point compositions are difficult to identify with good accuracy. Reported values vary up to 10% for even well-studied systems. Here, a technique is presented for high-precision determination of the critical composition of a partially miscible binary liquid system. Ninety-degree laser light-scattering intensities from single-phase samples are analyzed using an equation derived from nonclassical power laws and the pseudospinodal approximation. Results are reported for four liquid-liquid systems (aniline + hexane, isobutyric acid + water, methanol + cyclohexane, and methanol + carbon disulfide). Compared to other methods, the 90∘ light-scattering approach has a strong dependence on composition near the critical point, is less affected by temperature fluctuations, and is insensitive to the presence of trace impurities in the samples. Critical compositions found with 90∘ light scattering are precise to the parts-per-thousand level and show long-term reproducibility.
Determination of liquid-liquid critical point composition using 90^{∘} laser light scattering.
Williamson, J Charles; Brown, Allison M; Helvie, Elise N; Dean, Kevin M
2016-04-01
Despite over a century of characterization efforts, liquid-liquid critical point compositions are difficult to identify with good accuracy. Reported values vary up to 10% for even well-studied systems. Here, a technique is presented for high-precision determination of the critical composition of a partially miscible binary liquid system. Ninety-degree laser light-scattering intensities from single-phase samples are analyzed using an equation derived from nonclassical power laws and the pseudospinodal approximation. Results are reported for four liquid-liquid systems (aniline + hexane, isobutyric acid + water, methanol + cyclohexane, and methanol + carbon disulfide). Compared to other methods, the 90^{∘} light-scattering approach has a strong dependence on composition near the critical point, is less affected by temperature fluctuations, and is insensitive to the presence of trace impurities in the samples. Critical compositions found with 90^{∘} light scattering are precise to the parts-per-thousand level and show long-term reproducibility.
Konoshonkin, Alexander V.; Kustova, Natalia V.; Borovoi, Anatoli G.
2015-10-01
The open-source beam-splitting code is described which implements the geometric-optics approximation to light scattering by convex faceted particles. This code is written in C++ as a library which can be easy applied to a particular light scattering problem. The code uses only standard components, that makes it to be a cross-platform solution and provides its compatibility to popular Integrated Development Environments (IDE's). The included example of solving the light scattering by a randomly oriented ice crystal is written using Qt 5.1, consequently it is a cross-platform solution, too. Both physical and computational aspects of the beam-splitting algorithm are discussed. Computational speed of the beam-splitting code is obviously higher compared to the conventional ray-tracing codes. A comparison of the phase matrix as computed by our code with the ray-tracing code by A. Macke shows excellent agreement.
Sharma, S. K.
2012-12-01
A number of experimental elastic light scattering studies have been performed in the past few years with the aim of developing automated in vivo tools for differentiating a healthy red blood cell from a Plasmodium falciparum infected cell. This paper examines some theoretical aspects of the problem. An attempt has been made to simulate the scattering patterns of healthy as well as infected individual red blood cells. Two models, namely, a homogeneous sphere model and a coated sphere model have been considered. The scattering patterns predicted by these models are examined. A possible method for discriminating infected red blood cells from healthy ones has been suggested.
[Multiple scattering of visible and infrared light by sea fog over wind driving rough sea surface].
Sun, Xian-Ming; Wang, Hai-Hua; Lei, Cheng-Xin; Shen, Jin
2013-08-01
The present paper is concerned with computing the multiple scattering characteristics of a sea fog-sea surface couple system within this context. The single scattering characteristics of sea fog were studied by Mie theory, and the multiple scattering of sunlight by single sea fog layer was studied by radiative transfer theory. The reflection function of a statistically rough ocean surface was obtained using the standard Kirchhoff formulation, with shadowing effects taken into account. The reflection properties of the combined sea fog and ocean surface were obtained employing the adding method, and the results indicated that the reflected light intensity of sea fog increased with the sea background.
Analytic height correlation function of rough surfaces derived from light scattering
Zamani, M; Fazeli, S M; Downer, M C; Jafari, G R
2015-01-01
We obtain an analytic expression for the height correlation function of a rough surface based on the inverse wave scattering method of Kirchhoff theory. The expression directly relates the height correlation function to diffuse scattered intensity. We test the solution by measuring the angular distribution of light scattered from rough silicon surfaces, solving for the height correlation functions, and comparing them to functions derived from AFM measurements. The results show good agreement. The advantages of this method are its accurate analytical equation for the height correlation function and the simplicity of the experimental setup required to measure it.
Etxebarria, J; Ortega, J; Folcia, C L; Sanz-Enguita, G; Aramburu, I
2015-04-01
We have studied the degradation process of the laser emission in a cholesteric liquid crystal laser. We have found that there exists a negative correlation between the laser efficiency and the amount of light scattered by the liquid-crystal sample in the illuminated area. The growth of scattering is attributed to the appearance of small imperfections generated in the sample as a result of certain thermal processes that involve the dye molecules. The scattering implies an increase of the coefficient of distributed losses, which is the main response of the rise of the laser threshold.
Temporal intensity correlation of light scattered by a hot atomic vapor
Dussaux, A; Guerin, W; Alibart, O; Tanzilli, S; Vakili, F; Kaiser, R
2016-01-01
We present temporal intensity correlation measurements of light scattered by a hot atomic vapor. Clear evidence of photon bunching is shown at very short time-scales (ns) imposed by the Doppler broadening of the hot vapor. Moreover, we demonstrate that some relevant information about the scattering process, such as the ratio of single to multiple scattering, can be deduced from the measured intensity correlation function. These measurements confirm the interest of temporal intensity correlation measurements to access non-trivial spectral features, with potential applications in astrophysics.
Theoretical Models of Light Scattering Applied in Sizing Particles in Coal Water Slurry
Institute of Scientific and Technical Information of China (English)
王仁哲; 张荣曾; 徐志强
2004-01-01
Advantges and disadvantage of Mie scattering model and Fraunhofer diffraction model are discussed. The result shows that 1) the Fraunhofer diffraction model is simple in design and fast in operation, which is quite suitable for on-line control and 2) the intensity and energy distribution of diffracted light of both the Mie scattering model and the Fraunhofer theoretical model are compared and researched. Feasibility of using the Fraunhofer diffraction model to replace the Mie scattering model in measuring particles in coal water slurry is demonstrated.
Self-induced light trapping in nonlinear Fabry-Perot resonators
Pichugin, K. N.; Sadreev, A. F.
2016-10-01
In the framework of the coupled mode theory we consider light trapping between two off-channel resonators which serve as self-adjusted Fano mirrors due to the Kerr effect. By inserting an auxiliary nonlinear resonator between the mirrors we achieve self-tuning of phase shift between the mirrors. That allows for the light trapping for arbitrary distance between the mirrors.
Park, Sohee; Shin, Yongjin; Oh, Kwanghwan; Bang, Taehwan
2016-04-01
In flat-type light-emitting-diode (LED) lighting systems, a planar light is formed using a luminance source positioned on the side of the system and light guide panel (LGP) or reflecting plates. Thus, such systems are favorable for their thinness, which allows a relatively small number of LEDs to be used. However, the application of a high-power LED light to a large-area lighting system yields Lambertian luminaires; therefore, a point or a discomfort glare is produced, which generally causes degradation of the luminance efficiency and uniformity. In this study, we solved the problems of luminance non-uniformity and inefficiency by adjusting the orientation of an applied LGP scattered pattern and removing the remaining glare. Through computer simulation, optical characteristics that increase the efficiency even in the case of low-output LEDs were found. Specifically, a scattered pattern vertically oriented relative to the direction of the incident light improves the luminance uniformity at the side of the system, while a scattered pattern oriented parallel to the direction of the incident light plays the role of a waveguide. We implemented a flat-type LED lighting system by fabricating a large-area LGP based on the computer-simulation results and using an extremely sensitive laser. The optical characteristics observed using the laser-processed LGP were identical to those obtained in the computer simulation. Therefore, for large-area flat-type LED lighting systems, we confirmed that adjusting the orientation of the LGP scattered pattern can increase the luminance efficiency and uniformity.
Liu, Zhengwen; Liu, Shaopu; Wang, Lei; Peng, Juanjuan; He, Youqiu
2009-09-01
In pH 6.6 Britton-Robinson buffer medium, the CdS quantum dots capped by thioglycolic acid could react with aminoglycoside (AGs) antibiotics such as neomycin sulfate (NEO) and streptomycin sulfate (STP) to form the large aggregates by virtue of electrostatic attraction and the hydrophobic force, which resulted in a great enhancement of resonance Rayleigh scattering (RRS) and resonance non-linear scattering such as second-order scattering (SOS) and frequency doubling scattering (FDS). The maximum scattering peak was located at 310 nm for RRS, 568 nm for SOS and 390 nm for FDS, respectively. The enhancements of scattering intensity (Δ I) were directly proportional to the concentration of AGs in a certain ranges. A new method for the determination of trace NEO and STP using CdS quantum dots probe was developed. The detection limits (3 σ) were 1.7 ng mL -1 (NEO) and 4.4 ng mL -1 (STP) by RRS method, were 5.2 ng mL -1 (NEO) and 20.9 ng mL -1 (STP) by SOS method and were 4.4 ng mL -1 (NEO) and 25.7 ng mL -1 (STP) by FDS method, respectively. The sensitivity of RRS method was the highest. The optimum conditions and influence factors were investigated. In addition, the reaction mechanism was discussed.
Liu, Gang; Jayathilake, Pahala Gedara; Khoo, Boo Cheong
2014-02-01
Two nonlinear models are proposed to investigate the focused acoustic waves that the nonlinear effects will be important inside the liquid around the scatterer. Firstly, the one dimensional solutions for the widely used Westervelt equation with different coordinates are obtained based on the perturbation method with the second order nonlinear terms. Then, by introducing the small parameter (Mach number), a dimensionless formulation and asymptotic perturbation expansion via the compressible potential flow theory is applied. This model permits the decoupling between the velocity potential and enthalpy to second order, with the first potential solutions satisfying the linear wave equation (Helmholtz equation), whereas the second order solutions are associated with the linear non-homogeneous equation. Based on the model, the local nonlinear effects of focused acoustic waves on certain volume are studied in which the findings may have important implications for bubble cavitation/initiation via focused ultrasound called HIFU (High Intensity Focused Ultrasound). The calculated results show that for the domain encompassing less than ten times the radius away from the center of the scatterer, the non-linear effect exerts a significant influence on the focused high intensity acoustic wave. Moreover, at the comparatively higher frequencies, for the model of spherical wave, a lower Mach number may result in stronger nonlinear effects.
Light scattering by subwavelength Cu2O particles
Ullah, Kaleem; Liu, Xuefeng; Yadav, N. P.; Habib, Muhammad; Song, Li; García-Cámara, Braulio
2017-03-01
Novel metamaterials with new capabilities to manipulate light may be used by considering basic building blocks with new optical properties. This is the case with resonant magneto-dielectric particles. In this work, the resonant response of a high-dielectric Cu2O subwavelength particle is analyzed, both analytically and experimentally. The emergence of electric and magnetic resonances and their interferential effects, producing directional behaviors, can be used in a new generation of metamaterials, as well as new integrated optical devices.
Wahle, Chris W; Ross, David S; Thurston, George M
2013-09-28
We extend methods of solution of a light scattering partial differential equation for the free energy of mixing to apply to connected, isotropic ternary liquid composition domains that do not touch all three binary axes. To do so we mathematically analyze the problem of inferring needed Dirichlet boundary data, and solving for the free energy, with use of hypothetical static light scattering measurements that correspond to dielectric composition gradient vectors that have distinct directions. The physical idea behind the technique is that contrasting absorption properties of mixture components can result in such distinctly directed dielectric composition gradient vectors, due to their differing wavelength dependences of dielectric response. At suitably chosen wavelengths, contrasting light scattering efficiency patterns in the ternary composition triangle can then correspond to the same underlying free energy, and enlarge the scope of available information about the free energy, as shown here. We show how to use distinctly directed dielectric gradients to measure the free energy on both straight lines and curves within the ternary composition triangle, so as to provide needed Dirichlet conditions for light scattering partial differential equation solution. With use of Monte Carlo simulations of noisy light scattering data, we provide estimates of the overall system measurement time and sample spacing needed to determine the free energy to a desired degree of accuracy, for various angles between the assumed dielectric gradient vectors, and indicate how the measurement time depends on instrumental throughput parameters. The present analysis methods provide a way to use static light scattering to measure, directly, mixing free energies of many systems that contain such restricted liquid domains, including aqueous solutions of biological macromolecules, micellar mixtures and microemulsions, and many small molecule systems that are important in separation technology.
Blood cell counting and classification by nonflowing laser light scattering method
Yang, Ye; Zhang, Zhenxi; Yang, Xinhui; Jiang, Dazong; Yeo, Joon Hock
1999-11-01
A new non-flowing laser light scattering method for counting and classifying blood cells is presented. A linear charge- coupled device with 1024 elements is used to detect the scattered light intensity distribution of the blood cells. A pinhole plate is combined with the CCD to compete the focusing of the measurement system. An isotropic sphere is used to simulate the blood cell. Mie theory is used to describe the scattering of blood cells. In order to inverse the size distribution of blood cells from their scattered light intensity distribution, Powell method combined with precision punishment method is used as a dependent model method for measurement red blood cells and blood plates. Non-negative constraint least square method combined with Powell method and precision punishment method is used as an independent model for measuring white blood cells. The size distributions of white blood cells and red blood cells, and the mean diameter of red blood cells are measured by this method. White blood cells can be divided into three classes: lymphocytes, middle-sized cells and neutrocytes according to their sizes. And the number of blood cells in unit volume can also be measured by the linear dependence of blood cells concentration on scattered light intensity.