LWR high burn-up operation and MOX introduction. Fuel cycle performance from the viewpoint of waste management

International Nuclear Information System (INIS)

Inagaki, Yaohiro; Iwasaki, Tomohiko; Niibori, Yuichi; Sato, Seichi; Ohe, Toshiaki; Kato, Kazuyuki; Torikai, Seishi; Nagasaki, Shinya; Kitayama, Kazumi

2009-01-01

From the viewpoint of waste management, a quantitative evaluation of LWR nuclear fuel cycle system performance was carried out, considering both higher burn-up operation of UO 2 fuel coupled with the introduction of MOX fuel. A major parameter to quantify this performance is the number of high-level waste (HLW) glass units generated per GWd (gigawatt-day based on reactor thermal power generation before electrical conversion). This parameter was evaluated for each system up to a maximum burn-up of 70GWd/THM (gigawatt-day per ton of heavy metal) assuming current conventional reprocessing and vitrification conditions where the waste loading of glass is restricted by the heat generation rate, the MoO 3 content, or the noble metal content. The results showed that higher burn-up operation has no significant influence on the number of glass units generated per GWd for UO 2 fuel, though the number of glass units per THM increases linearly with burn-up and is restricted by the heat generation rate. On the other hand, the introduction of MOX fuel causes the number of glass units per GWd to double owing to the increase in the heat generation rate. An extended cooling period of the spent fuel prior to reprocessing effectively reduces the heat generation rate for UO 2 fuel, while a separation of minor actinides (Np, Am, and Cm) from the high-level waste provides additional reduction for MOX fuel. However, neither of these leads to a substantial reduction in the number of glass units, since the MoO 3 content or the noble metal content restricts the number of glass units rather than the heat generation rate. These results suggest that both the MoO 3 content and the noble metal content provide the key to reducing the amount of waste glass that is generated, leading to an overall improvement in fuel cycle system performance. (author)

Mox fuel experience: present status and future improvements

International Nuclear Information System (INIS)

Blanpain, P.; Chiarelli, G.

2001-01-01

Up to December 2000, more than 1700 MOX fuel assemblies have been delivered by Framatome ANP/Fragema to 20 French, 2 Belgian and 3 German PWRs. More than 1000 MOX fuel assemblies have been delivered by Framatome ANP GmbH (formerly Siemens) to 11 German PWRs and BWRs and to 3 Swiss PWRs. Operating MOX fuel up to discharge burnups of about 45,000 MWd/tM is done without any penalty on core operating conditions and fuel reliability. Performance data for fuel and materials have been obtained from an outstanding surveillance program. The examinations have concluded that there have been no significant differences in MOX fuel assembly characteristics relative to UO 2 fuel. The data from these examinations, combined with a comprehensive out-of-core and in-core analytical test program on the current fuel products, are being used to confirm and upgrade the design models necessary for the continuing improvement of the MOX product. As MOX fuel has reached a sufficient maturity level, the short term step is the achievement of the parity between UO 2 and MOX fuels in the EdF French reactors. This involves a single operating scheme for both fuels with an annual quarter core reload type and an assembly discharge burnup goal of 52,000 MWd/tM. That ''MOX parity'' product will use the AFA-3G assembly structure which will increase the fuel rod design margins with regards to the end-of-life internal pressure criteria. But the fuel development objective is not limited to the parity between the current MOX and UO 2 products: that parity must remain guaranteed and the MOX fuel managements must evolve in the same way as the UO 2 ones. The goal of the MOX product development program underway in France is the demonstration over the next ten years of a fuel capable of reaching assembly burnups of 70,000 MWd/tM. (author)

Development of ORIGEN libraries for mixed oxide (MOX) fuel assembly designs

International Nuclear Information System (INIS)

Mertyurek, Ugur; Gauld, Ian C.

2016-01-01

Highlights: • ORIGEN MOX library generation process is described. • SCALE burnup calculations are validated against measured MOX fuel samples from the MALIBU program. • ORIGEN MOX libraries are verified using the OECD Phase IV-B benchmark. • There is good agreement for calculated-to-measured isotopic distributions. - Abstract: ORIGEN cross section libraries for reactor-grade mixed oxide (MOX) fuel assembly designs have been developed to provide fast and accurate depletion calculations to predict nuclide inventories, radiation sources and thermal decay heat information needed in safety evaluations and safeguards verification measurements of spent nuclear fuel. These ORIGEN libraries are generated using two-dimensional lattice physics assembly models that include enrichment zoning and cross section data based on ENDF/B-VII.0 evaluations. Using the SCALE depletion sequence, burnup-dependent cross sections are created for selected commercial reactor assembly designs and a representative range of reactor operating conditions, fuel enrichments, and fuel burnup. The burnup dependent cross sections are then interpolated to provide problem-dependent cross sections for ORIGEN, avoiding the need for time-consuming lattice physics calculations. The ORIGEN libraries for MOX assembly designs are validated against destructive radiochemical assay measurements of MOX fuel from the MALIBU international experimental program. This program included measurements of MOX fuel from a 15 × 15 pressurized water reactor assembly and a 9 × 9 boiling water reactor assembly. The ORIGEN MOX libraries are also compared against detailed assembly calculations from the Phase IV-B numerical MOX fuel burnup credit benchmark coordinated by the Nuclear Energy Agency within the Organization for Economic Cooperation and Development. The nuclide compositions calculated by ORIGEN using the MOX libraries are shown to be in good agreement with other physics codes and with experimental data.

Validation of a new continuous Monte Carlo burnup code using a Mox fuel assembly

International Nuclear Information System (INIS)

El bakkari, B.; El Bardouni, T.; Merroun, O.; El Younoussi, C.; Boulaich, Y.; Boukhal, H.; Chakir, E.

2009-01-01

The reactivity of nuclear fuel decreases with irradiation (or burnup) due to the transformation of heavy nuclides and the formation of fission products. Burnup credit studies aim at accounting for fuel irradiation in criticality studies of the nuclear fuel cycle (transport, storage, etc...). The principal objective of this study is to evaluate the potential capabilities of a newly developed burnup code called 'BUCAL1'. BUCAL1 differs in comparison with other burnup codes as it does not use the calculated neutron flux as input to other computer codes to generate the nuclide inventory for the next time step. Instead, BUCAL1 directly uses the neutron reaction tally information generated by MCNP for each nuclide of interest to determine the new nuclides inventory. This allows the full capabilities of MCNP to be incorporated into the calculation and a more accurate and robust analysis to be performed. Validation of BUCAL1 was processed by code-to-code comparisons using predictions of several codes from the NEA/OCED. Infinite multiplication factors (k ∞ ) and important fission product and actinide concentrations were compared for a MOX core benchmark exercise. Results of calculations are analysed and discussed.

Thermal property change of MOX and UO{sub 2} irradiated up to high burnup of 74 GWd/t

Energy Technology Data Exchange (ETDEWEB)

Nakae, Nobuo, E-mail: nakae-nobuo@jnes.go.jp [Japan Nuclear Energy Safety Organization (JNES), Toranomon Towers Office, 4-1-28, Toranomon, Minato-ku, Tokyo 105-0001 (Japan); Akiyama, Hidetoshi; Miura, Hiromichi; Baba, Toshikazu; Kamimura, Katsuichiro [Japan Nuclear Energy Safety Organization (JNES), Toranomon Towers Office, 4-1-28, Toranomon, Minato-ku, Tokyo 105-0001 (Japan); Kurematsu, Shigeru; Kosaka, Yuji [Nuclear Development Corporation (NDC), 622-12, Funaishikawa, Tokai-mura, Ibaraki 319-1111 (Japan); Yoshino, Aya; Kitagawa, Takaaki [Mitsubishi Nuclear Fuel Co., LTD. (MNF), 12-1, Yurakucho 1-Chome, Chiyoda-ku, Tokyo 100-0006 (Japan)

2013-09-15

Thermal property is important because it controls fuel behavior under irradiation. The thermal property change at high burnup of more than 70 GWd/t is examined. Two kinds of MOX fuel rods, which were fabricated by MIMAS and SBR methods, and one referenced UO{sub 2} fuel rod were used in the experiment. These rods were taken from the pre-irradiated rods (IFA 609/626, of which irradiation test were carried out by Japanese PWR group) and re-fabricated and re-irradiated in HBWR as IFA 702 by JNES. The specification of fuel corresponds to that of 17 × 17 PWR type fuel and the axially averaged linear heat rates (LHR) of MOX rods are 25 kW/m (BOL of IFA 702) and 20 kW/m (EOL of IFA 702). The axial peak burnups achieved are about 74 GWd/t for both of MOX and UO{sub 2}. Centerline temperature and plenum gas pressure were measured in situ during irradiation. The measured centerline temperature is plotted against LHR at the position where thermocouples are fixed. The slopes of MOX are corresponded to each other, but that of UO{sub 2} is higher than those of MOX. This implies that the thermal conductivity of MOX is higher than that of UO{sub 2} at high burnup under the condition that the pellet–cladding gap is closed during irradiation. Gap closure is confirmed by the metallography of the postirradiation examinations. It is understood that thermal conductivity of MOX is lower than that of UO{sub 2} before irradiation since phonon scattering with plutonium in MOX becomes remarkable. A phonon scattering with plutonium decreases in MOX when burnup proceeds. Thus, thermal conductivity of MOX becomes close to that of UO{sub 2}. A reverse phenomenon is observed at high burnup region. The phonon scattering with fission products such as Nd and Zr causes a degradation of thermal conductivity of burnt fuel. It might be speculated that this scattering effect causes the phenomenon and the mechanism is discussed here.

Chemical analyses and calculation of isotopic compositions of high-burnup UO{sub 2} fuels and MOX fuels

Energy Technology Data Exchange (ETDEWEB)

Matsumura, Tetsuo; Sasahara, Akihiro [Central Research Inst. of Electric Power Industry, Tokyo (Japan)

2001-08-01

Chemical analysis activities of isotopic compositions of high-burnup UO{sub 2} fuels and MOX fuels in CRIEPI and calculation evaluation are reviewed briefly. C/E values of ORIGEN2, in which original libraries and JENDL-3.2 libraries are used, and other codes with chemical analysis data are reviewed and evaluated. Isotopic compositions of main U and Pu in fuels can be evaluated within 10% relative errors by suitable libraries and codes. Void ratio is effective parameter for C/E values in BWR fuels. JENDL-3.2 library shows remarkable improvement compared with original libraries in isotopic composition evaluations of FP nuclides. (author)

Micro-Reactor Physics of MOX-Fueled Core

International Nuclear Information System (INIS)

Takeda, T.

2001-01-01

Recently, fuel assemblies of light water reactors have become complicated because of the extension of fuel burnup and the use of high-enriched Gd and mixed-oxide (MOX) fuel, etc. In conventional assembly calculations, the detailed flux distribution, spectrum distribution, and space dependence of self-shielding within a fuel pellet are not directly taken into account. The experimental and theoretical study of investigating these microscopic properties is named micro-reactor physics. The purpose of this work is to show the importance of micro-reactor physics in the analysis of MOX fuel assemblies. Several authors have done related studies; however, their studies are limited to fuel pin cells, and they are never mentioned with regard to burnup effect, which is important for actual core design

Effect of Pu-rich agglomerate in MOX fuel on a lattice calculation

International Nuclear Information System (INIS)

Kawashima, Katsuyuki; Yamamoto, Toru; Namekawa, Masakazu

2007-01-01

The effect of Pu-rich agglomerates in U-Pu mixed oxide (MOX) fuel on a lattice calculation has been demonstrated. The Pu-rich agglomerate parameters are defined based on the measurement data of MIMAS-MOX and the focus is on the highly enriched MOX fuel in accordance with increased burnup resulting in a higher volume fraction of the Pu-rich agglomerates. The lattice calculations with a heterogeneous fuel model and a homogeneous fuel model are performed simulating the PWR 17x17 fuel assembly. The heterogeneous model individually treats the Pu-rich agglomerate and U-Pu matrix, whereas the homogeneous model homogenizes the compositions within the fuel pellet. A continuous-energy Monte Carlo burnup code, MVP-BURN, is used for burnup calculations up to 70 GWd/t. A statistical geometry model is applied in modeling a large number of Pu-rich agglomerates assuming that they are distributed randomly within the MOX fuel pellet. The calculated nuclear characteristics include k-inf, Pu isotopic compositions, power density and burnup of the Pu-rich agglomerates, as well as the pellet-averaged Pu compositions as a function of burnup. It is shown that the effect of Pu-rich agglomerates on the lattice calculation is negligibly small. (author)

Status of irradiation testing and PIE of MOX (Pu-containing) fuel

International Nuclear Information System (INIS)

Dimayuga, F.C.; Zhou, Y.N.; Ryz, M.A.

1995-01-01

This paper describes AECL's mixed oxide (MOX) fuel-irradiation and post-irradiation examination (PIE) program. Post-irradiation examination results of two major irradiation experiments involving several (U, Pu)O 2 fuel bundles are highlighted. One experiment involved bundles irradiated to burnups ranging fro 400 to 1200 MWh/kgHe in the Nuclear Power Demonstration (NPD) reactor. The other experiment consisted of several (U, Pu)O 2 bundles irradiated to burnups of up to 500 Mwh/kgHe in the National Research Universal (NRU) reactor. Results of these experiments demonstrate the excellent performance of CANDU MOX fuel. This paper also outlines the status of current MOX fuel irradiation tests, including the irradiation of various (U, Pu)O 2 bundles. The strategic importance of MOX fuel to CANDU fuel-cycle flexibility is discussed. (author)

MOX fuel design and development consideration

International Nuclear Information System (INIS)

Yamate, K.; Abeta, S.; Suzuki, K.; Doi, S.

1997-01-01

Pu thermal utilization in Japan will be realized in several plants in late 1990's, and will be expanded gradually. For this target, adequacy of methods for MOX fuel design, nuclear design, and safety analysis has been evaluated by the committee of competent authorities organized by government in advance of the licensing application. There is no big difference of physical properties and irradiation behaviors between MOX fuel and UO 2 fuel, because Pu content of MOX fuel for Pu thermal utilization is low. The fuel design code for UO 2 fuel will be applied with some modifications, taking into account of characteristic of MOX fuel. For nuclear design, new code system is to be applied to treat the heterogeneity in MOX fuel assembly and the neutron spectrum interaction with UO 2 fuel more accurately. For 1/3 MOX fueled core in three loop plant, it was confirmed that the fuel rod mechanical design could meet the design criteria, with slight reduction of initial back-fitting pressure, and with appropriate fuel loading patterns in the core to match power with UO 2 fuel. With the increase of MOX fuel fraction in the core, control rod worth and boron worth decrease. Compensating the decrease by adding control rod and utilizing enriched B-10 in safety injection system, 100% MOX fueled core could be possible. Up to 1/3 MOX fueled core in three loop plant, no such modifications of the plant is necessary. The fraction of MOX fuel in PWR is designed to less than 1/3 in the present program. In order to improve Pu thermal utilization in future, various R and D program on fuel design and nuclear design are being performed, such as the irradiation program of MOX fuel manufactured through new process to the extent of high burnup. (author). 8 refs, 9 figs, 2 tabs

Burnup effect on nuclear fuel cycle cost using an equilibrium model

International Nuclear Information System (INIS)

Youn, S. R.; Kim, S. K.; Ko, W. I.

2014-01-01

The degree of fuel burnup is an important technical parameter to the nuclear fuel cycle, being sensitive and progressive to reduce the total volume of process flow materials and eventually cut the nuclear fuel cycle costs. This paper performed the sensitivity analysis of the total nuclear fuel cycle costs to changes in the technical parameter by varying the degree of burnups in each of the three nuclear fuel cycles using an equilibrium model. Important as burnup does, burnup effect was used among the cost drivers of fuel cycle, as the technical parameter. The fuel cycle options analyzed in this paper are three different fuel cycle options as follows: PWR-Once Through Cycle(PWR-OT), PWR-MOX Recycle, Pyro-SFR Recycle. These fuel cycles are most likely to be adopted in the foreseeable future. As a result of the sensitivity analysis on burnup effect of each three different nuclear fuel cycle costs, PWR-MOX turned out to be the most influenced by burnup changes. Next to PWR-MOX cycle, in the order of Pyro-SFR and PWR-OT cycle turned out to be influenced by the degree of burnup. In conclusion, the degree of burnup in the three nuclear fuel cycles can act as the controlling driver of nuclear fuel cycle costs due to a reduction in the volume of spent fuel leading better availability and capacity factors. However, the equilibrium model used in this paper has a limit that time-dependent material flow and cost calculation is impossible. Hence, comparative analysis of the results calculated by dynamic model hereafter and the calculation results using an equilibrium model should be proceed. Moving forward to the foreseeable future with increasing burnups, further studies regarding alternative material of high corrosion resistance fuel cladding for the overall

Increased fuel burn-up and fuel cycle equilibrium

International Nuclear Information System (INIS)

Debes, M.

2001-01-01

Improvement of nuclear competitiveness will rely mainly on increased fuel performance, with higher burn-up, and reactors sustained life. Regarding spent fuel management, the EDF current policy relies on UO 2 fuel reprocessing (around 850 MTHM/year at La Hague) and MOX recycling to ensure plutonium flux adequacy (around 100 MTHM/year, with an electricity production equivalent to 30 TWh). This policy enables to reuse fuel material, while maintaining global kWh economy with existing facilities. It goes along with current perspective to increase fuel burn-up up to 57 GWday/t mean in 2010. The following presentation describes the consequences of higher fuel burn-up on fuel cycle and waste management and implementation of a long term and global equilibrium for decades in spent fuel management resulting from this strategy. (author)

Optimization of MOX fuel cycles in pebble bed HTGR

International Nuclear Information System (INIS)

Wei Jinfeng; Li Fu; Sun Yuliang

2013-01-01

Compared with light water reactor (LWR), the pebble bed high temperature gas-cooled reactor (HTGR) is able to operate in a full mixed oxide (MOX) fuelled core without significant change to core structure design. Based on a reference design of 250 MW pebble bed HTGR, four MOX fuel cycles were designed and evaluated by VSOP program package, including the mixed Pu-U fuel pebbles and mixed loading of separate Pu-pebbles and U-pebbles. Some important physics features were investigated and compared for these four cycles, such as the effective multiplication factor of initial core, the pebble residence time, discharge burnup, and temperature coefficients. Preliminary results show that the overall performance of one case is superior to other equivalent MOX fuel cycles on condition that uranium fuel elements and plutonium fuel elements are separated as the different fuel pebbles and that the uranium fuel elements are irradiated longer in the core than the plutonium fuel elements, and the average discharge burnup of this case is also higher than others. (authors)

Evaluation of the characteristics of uranium and plutonium Mixed Oxide (MOX) fuel

Energy Technology Data Exchange (ETDEWEB)

NONE

2013-08-15

MOX fuel irradiation test up to high burnup has been performed for five years. Irradiation test of MOX fuel having high plutonium content has also been performed from JFY 2007 and it still continues. A lot of irradiation data have been obtained through these tests. The activities done in JFY 2012 are mainly focused on Post Irradiation Examination (PIE) data analysis concerning thermal property change and fission gas release. In the former work thermal conductivity degradation due to burnup is examined and in the latter work the dependence of fission gas release mechanism on fuel pellet microstructure is examined. This report mainly covers the result of analysis. It is found that thermal conductivity degradation of MOX fuel due to burnup is less than that of UO{sub 2} fuel and that fission gas release mechanism of high enriched fissile zone (so called Pu spot) is much different from that of low enriched fissile zone (so called Matrix). (author)

Burning of MOX fuels in LWRs; fuel history effects on thermal properties of hull and end piece wastes and the repository performance

International Nuclear Information System (INIS)

Hirano, Fumio; Sato, Seichi; Kozaki, Tamotsu

2012-01-01

The thermal impacts of hull and end piece wastes from the reprocessing of MOX spent fuels burned in LWRs on repository performance were investigated. The heat generation rates in MOX spent fuels and the resulting heat generation rates in hull and end piece wastes change depending on the history of MOX fuels. This history includes the burn-up of UO 2 spent fuels from which the Pu is obtained, the cooling period before reprocessing, the storage period of fresh MOX fuels before being loaded into an LWR, as well as the burn-up of the MOX fuels. The heat generation rates in hull and end piece wastes from the reprocessing of MOX spent fuels with any of those histories are significantly larger than those from UO 2 spent fuels with burn-ups of 45 GWd/THM. If a temperature below 80degC is specified for cement-based materials used in waste packages after disposal, the allowable number of canisters containing compacted hull and end pieces in a package for 45 and 70 GWd-MOX needs to be limited to a value of 0.4-1.6, which is significantly lower than 4.0 for 45 GWd-UO 2 . (author)

Full MOX high burn-up PWR

Energy Technology Data Exchange (ETDEWEB)

Okubo, Tsutomu; Kugo, Teruhiko; Shimada, Shoichiro; Araya, Fumimasa; Ochiai, Masaaki [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

1999-12-01

As a part of conceptual investigation on advanced light water reactors for the future, a light water reactor with the high burn-up of 100 GWd/t, the long cycle operation of 3 years and the full MOX core is being studied, aiming at the improvement on economical aspects, the reduction of the spent fuel production, the utilization of Plutonium and so forth. The present report summarizes investigation on PWR-type reactors. The core with the increased moderation of the moderator-to-fuel volume ratio of 2.6 {approx} 3.0 has been proposed be such a core that accomplishes requirements mentioned above. Through the neutronic and the thermo-hydrodynamic evaluation, the performances of the core have been evaluated. Also, the safety designing is underway considering the reactor system with the passive safety features. (author)

gamma-ray spectra measurements for long cooled MOX spent fuels

International Nuclear Information System (INIS)

Murakami, Kiyonobu; Kobayashi, Iwao

1993-09-01

Gamma-ray spectra of spent fuels have important informations in the estimation of burnup rate, concentration of fission products, cooling time and etc. which are required in the fuel loading control of reactors and special nuclear materials accountancy from the view point of safe guard. Although, some available data are given about uranium dioxide fuels, few data are given about uranium and plutonium dioxide mixtures (MOX fuels). Especially, there is few data about MOX fuels which are irradiated in thermal reactors and cooled more than ten years. Gamma-ray spectra are measured for PuO 2 -UO 2 fuel rods (IFA-159, IFA-160) which are irradiated at HBWR in Norway up to 9,420 and 5,340MWd/t respectively. Gamma-ray spectra had been measured about the two fuels ten years ago at the spent fuel pond of Japan Demonstration Reactor (JPDR). The objectives of this measurement is to know how decayed the gamma-ray spectra in these ten years and some fission products are there which are effective to estimate burnup rate of spent MOX fuels. (author)

Measurement of burnup in FBR MOX fuel irradiated to high burnup

International Nuclear Information System (INIS)

Koyama, Shin-ichi; Osaka, Masahiko; Sekine, Takashi; Morozumi, Katsufumi; Namekawa, Takashi; Itoh, Masahiko

2003-01-01

The burnup of fuel pins in the subassemblies irradiated at the range from 0.003 to 13.28% FIMA in the JOYO MK-II core were measured by the isotope dilution analysis. For the measurement, 75 and 51 specimens were taken from the fuel pins of driver fuel and irradiation test subassemblies, respectively. The data of burnup could be obtained within an experimental error of 4%, and were compared with the ones calculated by 3-dimensional neutron diffusion codes MAGI and ESPRIT-J, which are used for JOYO core management system. Both data of burnup almost agree with each other within an error of 5%. For the fuel pins loaded at the outer region of the subassembly in the 4th row, which was adjacent to reflectors, however, some of the calculation results were 15% less at most than the measured values. It is suggested from the calculation by a Monte Carlo code MCNP-4A that this difference between the calculated and the measured data attribute from the softening of neutron flux in the region adjacent to the reflector. (author)

MOX and UOX PWR fuel performances EDF operating experience

International Nuclear Information System (INIS)

Provost, Jean-Luc; Debes, Michel

2005-01-01

Based on a large program of experimentations implemented during the 90s, the industrial achievement of new FAs designs with increased performances opens up new prospects. The currently UOX fuels used on the 58 EDF PWR units are now authorized up to a maximum FA burn-up of 52 GWd/t with a large experience from 45 to 50 GWd/t. Today, the new products, along with the progress made in the field of calculation methods, still enable to increase further the fuel performances with respect to the safety margins. Thus, the conditions are met to implement in the next years new fuel managements on each NPPs series of the EDF fleet with increased enrichment (up to 4.5%) and irradiation limits (up to 62 GWd/t). The recycling of plutonium is part of EDF's reprocessing/recycling strategy. Up to now, 20 PWR 900 MW reactors are managed in MOX hybrid management. The feedback experience of 18 years of PWR operation with MOX is satisfactory, without any specific problem regarding manoeuvrability or plant availability. EDF is now looking to introduce MOX fuels with a higher plutonium content (up to 8.6%) equivalent to natural uranium enriched to 3.7%. It is the goal of the MOX Parity core management which achieve balance of MOX and UOX fuel performance with a significant increase of the MOX average discharge burn-up (BU max: 52 GWd/t for MOX and UOX). The industrial maturity of new FAs designs, with increased performances, allows the implementation in the next years of new fuel managements on each NPPs series of the EDF fleet. The scheduling of the implementation of the new fuel managements on the PWRs fleet is a great challenge for EDF, with important stakes: the nuclear KWh cost decrease with the improvement of the plant operation performance. (author)

Code Analyses Supporting PIE of Weapons-Grade MOX Fuel

International Nuclear Information System (INIS)

Ott, Larry J.; Bevard, Bruce Balkcom; Spellman, Donald J.; McCoy, Kevin

2010-01-01

The U.S. Department of energy has decided to dispose of a portion of the nation's surplus weapons-grade plutonium by reconstituting it into mixed oxide (MOX) fuel and irradiating the fuel in commercial power reactors. Four lead test assemblies (LTAs) were manufactured with weapons-grade mixed oxide (WG-MOX) fuel and irradiated in the Catawba Nuclear Station Unit 1, to a maximum fuel rod burnup of ∼47.3 GWd/MTHM. As part of the fuel qualification process, five rods with varying burnups and initial plutonium contents were selected from one assembly and shipped to the Oak Ridge National Laboratory (ORNL) for hot cell examination. ORNL has provided analytical support for the post-irradiation examination (PIE) of these rods via extensive fuel performance modeling which has aided in instrument settings and PIE data interpretation. The results of these fuel performance simulations are compared in this paper with available PIE data.

Overall models and experimental database for UO2 and MOX fuel increasing performance

International Nuclear Information System (INIS)

Bernard, L.C.; Blanpain, P.

2001-01-01

COPERNIC is an advanced fuel rod performance code developed by Framatome. It is based on the TRANSURANUS code that contains a clear and flexible architecture, and offers many modeling possibilities. The main objectives of COPERNIC are to accurately predict steady-state and transient fuel operations at high burnups and to incorporate advanced materials such as the Framatome M5-alloy cladding. An extensive development program was undertaken to benchmark the code to very high burnups and to new M5-alloy cladding data. New models were developed for the M5-alloy cladding and the COPERNIC thermal models were upgraded and improved to extend the predictions to burnups over 100 GWd/tM. Since key phenomena, like fission gas release, are strongly temperature dependent, many other models were upgraded also. The COPERNIC qualification range extends to 67, 55, 53 GWd/tM respectively for UO 2 , UO 2 -Gd 2 O 3 , and MOX fuels with Zircaloy-4 claddings. The range extends to 63 GWd/tM with UO 2 fuel and the advanced M5-alloy cladding. The paper focuses on thermal and fission gas release models, and on MOX fuel modeling. The COPERNIC thermal model consists of several submodels: gap conductance, gap closure, fuel thermal conductivity, radial power profile, and fuel rim. The fuel thermal conductivity and the gap closure models, in particular, have been significantly improved. The model was benchmarked with 3400 fuel centerline temperature data from many French and international programs. There are no measured to predicted statistical biases with respect to linear heat generation rate or burnup. The overall quality of the model is state-of-the-art as the model uncertainty is below 10 %. The fission gas release takes into account athermal and thermally activated mechanisms. The model was adapted to MOX and Gadolinia fuels. For the heterogeneous MOX MIMAS fuels, an effective burnup is used for the incubation threshold. For gadolinia fuels, a scaled temperature effect is used. The

Thermal conductivity degradation analyses of LWR MOX fuel by the quasi-two phase material model

International Nuclear Information System (INIS)

Kosaka, Yuji; Kurematsu, Shigeru; Kitagawa, Takaaki; Suzuki, Akihiro; Terai, Takayuki

2012-01-01

The temperature measurements of mixed oxide (MOX) and UO 2 fuels during irradiation suggested that the thermal conductivity degradation rate of the MOX fuel with burnup should be slower than that of the UO 2 fuel. In order to explain the difference of the degradation rates, the quasi-two phase material model is proposed to assess the thermal conductivity degradation of the MIMAS MOX fuel, which takes into account the Pu agglomerate distributions in the MOX fuel matrix as fabricated. As a result, the quasi-two phase model calculation shows the gradual increase of the difference with burnup and may expect more than 10% higher thermal conductivity values around 75 GWd/t. While these results are not fully suitable for thermal conductivity degradation models implemented by some industrial fuel manufacturers, they are consistent with the results from the irradiation tests and indicate that the inhomogeneity of Pu content in the MOX fuel can be one of the major reasons for the moderation of the thermal conductivity degradation of the MOX fuel. (author)

Burnup Credit of French PWR-MOx fuels: methodology and associated conservatisms with the JEFF-3.1.1 evaluation

International Nuclear Information System (INIS)

Chambon, A.

2013-01-01

Considering spent fuel management (storage, transport and reprocessing), the approach using 'fresh fuel assumption' in criticality-safety studies results in a significant conservatism in the calculated value of the system reactivity. The concept of Burnup Credit (BUC) consists in considering the reduction of the spent fuel reactivity due to its burnup. A careful BUC methodology, developed by CEA in association with AREVA-NC was recently validated and written up for PWR-UOx fuels. However, 22 of 58 French reactors use MOx fuel, so more and more irradiated MOx fuels have to be stored and transported. As a result, why industrial partners are interested in this concept is because taking into account this BUC concept would enable for example a load increase in several fuel cycle devices. Recent publications and discussions within the French BUC Working Group highlight the current interest of the BUC concept in PWR-MOx spent fuel industrial applications. In this case of PWR-MOx fuel, studies show in particular that the 15 FPs selected thanks to their properties (absorbing, stable, non-gaseous) are responsible for more than a half of the total reactivity credit and 80% of the FPs credit. That is why, in order to get a conservative and physically realistic value of the application k eff and meet the Upper Safety Limit constraint, calculation biases on these 15 FPs inventory and individual reactivity worth should be considered in a criticality-safety approach. In this context, thanks to an exhaustive literature study, PWR-MOx fuels particularities have been identified and by following a rigorous approach, a validated and physically representative BUC methodology, adapted to this type of fuel has been proposed, allowing to take fission products into account and to determine the biases related to considered isotopes inventory and to reactivity worth. This approach consists of the following studies: - isotopic correction factors determination to guarantee the criticality

Fabrication of MOX fuel element clusters for irradiation in PWL, CIRUS

International Nuclear Information System (INIS)

Roy, P.R.; Purushotham, D.S.C.; Majumdar, S.

1983-01-01

Three clusters, each containing 6 zircaloy-2 clad short length fuel elements of either MOX or UO 2 fuel pellets were fabricated for irradiation in pressurized water loop of CIRUS. The major objectives of the programme were: (a) to optimize the various fabrication parameters for developing a flow sheet for MOX fuel element fabrication; (b) to study the performance of the MOX fuel elements at a peak heat flux of 110 W/cm 2 ; and (c) to study the effect of various fuel pellet design changes on the behaviour of the fuel element under irradiation. Two clusters, one each of UO 2 and MOX, have been successfully irradiated to the required burn-up level and are now awaiting post irradiation examinations. The third MOX cluster is still undergoing irradiation. Fabrication of these fuel elements involved considerable amount of developing work related to the fabrication of the MOX fuel pellets and the element welding technique and is reported in detail in this report. (author)

Diametral strain of fast reactor MOX fuel pins with austenitic stainless steel cladding irradiated to high burnup

Energy Technology Data Exchange (ETDEWEB)

Uwaba, Tomoyuki, E-mail: uwaba.tomoyuki@jaea.go.jp [Japan Atomic Energy Agency, 4002, Narita-cho, Oarai-machi, Ibaraki 311-1393 (Japan); Ito, Masahiro; Maeda, Koji [Japan Atomic Energy Agency, 4002, Narita-cho, Oarai-machi, Ibaraki 311-1393 (Japan)

2011-09-30

Highlights: > We evaluated diametral strain of fast reactor MOX fuel pins irradiated to 130 GWd/t. > The strain was due to cladding void swelling and irradiation creep. > The irradiation creep was caused by internal gas pressure and PCMI. > The PCMI was associated with pellet swelling by rim structure or by cesium uranate. > The latter effect tended to increase the cumulative damage fraction of the cladding. - Abstract: The C3M irradiation test, which was conducted in the experimental fast reactor, 'Joyo', demonstrated that mixed oxide (MOX) fuel pins with austenitic steel cladding could attain a peak pellet burnup of about 130 GWd/t safely. The test fuel assembly consisted of 61 fuel pins, whose design specifications were similar to those of driver fuel pins of a prototype fast breeder reactor, 'Monju'. The irradiated fuel pins exhibited diametral strain due to cladding void swelling and irradiation creep. The cladding irradiation creep strain were due to the pellet-cladding mechanical interaction (PCMI) as well as the internal gas pressure. From the fuel pin ceramographs and {sup 137}Cs gamma scanning, it was found that the PCMI was associated with the pellet swelling which was enhanced by the rim structure formation or by cesium uranate formation. The PCMI due to cesium uranate, which occurred near the top of the MOX fuel column, significantly affected cladding hoop stress and thermal creep, and the latter effect tended to increase the cumulative damage fraction (CDF) of the cladding though the CDF indicated that the cladding still had some margin to failure due to the creep damage.

Burnup simulations of different fuel grades using the MCNPX Monte Carlo code

Directory of Open Access Journals (Sweden)

Asah-Opoku Fiifi

2014-01-01

Full Text Available Global energy problems range from the increasing cost of fuel to the unequal distribution of energy resources and the potential climate change resulting from the burning of fossil fuels. A sustainable nuclear energy would augment the current world energy supply and serve as a reliable future energy source. This research focuses on Monte Carlo simulations of pressurized water reactor systems. Three different fuel grades - mixed oxide fuel (MOX, uranium oxide fuel (UOX, and commercially enriched uranium or uranium metal (CEU - are used in this simulation and their impact on the effective multiplication factor (Keff and, hence, criticality and total radioactivity of the reactor core after fuel burnup analyzed. The effect of different clad materials on Keff is also studied. Burnup calculation results indicate a buildup of plutonium isotopes in UOX and CEU, as opposed to a decline in plutonium radioisotopes for MOX fuel burnup time. For MOX fuel, a decrease of 31.9% of the fissile plutonium isotope is observed, while for UOX and CEU, fissile plutonium isotopes increased by 82.3% and 83.8%, respectively. Keff results show zircaloy as a much more effective clad material in comparison to zirconium and stainless steel.

Isotopic analyses and calculation by use of JENDL-3.2 for high burn-up UO2 and MOX spent fuels

International Nuclear Information System (INIS)

Sasahara, Akihiro; Matsumura, Tetsuo; Nicolaou, G.; Betti, M.; Walker, C.T.

1997-01-01

The post irradiation examinations (PIE) were carried out for high burn-up UO 2 spent fuel (3.8%U235, average burn-up:60GWd/t) and mixed oxide (MOX) spent fuel (5.07%Pu, average burn-up:45GWd/t). The PIE includes, a) isotopic analysis, b) electron probe microanalysis (EPMA) in pellet cross section and so on. The results of isotopic analyses and EPMA were compared with ORIGEN2/82 and VIM-BURN calculation results. In VIM-BURN calculation, the nuclear data of actinides were proceeded from new data file, JENDL-3.2. The sensitivities of power history and moderator density to nuclides composition were investigated by VIM-BURN calculation and consequently power history mainly effected on Am241 and Am242m and moderator density effected on fissile nuclides. From EPMA results of U and Pu distribution in pellet, VIM-BURN calculation showed reasonable distribution in pellet cross section. (author)

Performance of cladding on MOX fuel with low 240Pu/239Pu ratio

International Nuclear Information System (INIS)

McCoy, K.; Blanpain, P.; Morris, R.

2015-01-01

The U.S. Department of Energy has decided to dispose of a portion of its surplus plutonium by reconstituting it into mixed oxide (MOX) fuel and irradiating it in commercial power reactors. As part of fuel qualification, four lead assemblies were manufactured and irradiated to a maximum fuel rod average burnup of 47.3 MWd/kg heavy metal. This was the world's first commercial irradiation of MOX fuel with a 240 Pu/ 239 Pu ratio less than 0.10. Five fuel rods with varying burnups and plutonium contents were selected from one of the assemblies and shipped to Oak Ridge National Laboratory for hot cell examination. This paper discusses the results of those examinations with emphasis on cladding performance. Exams relevant to the cladding included visual and eddy current exams, profilometry, microscopy, hydrogen analysis, gallium analysis, and mechanical testing. There was no discernible effect of the type of MOX fuel on the performance of the cladding. (authors)

The effect of dissolved hydrogen on the dissolution of 233U doped UO2(s) high burn-up spent fuel and MOX fuel

International Nuclear Information System (INIS)

Carbol, P.; Spahiu, K.

2005-03-01

In this report the results of the experimental work carried out in a large EU-research project (SFS, 2001-2004) on spent fuel stability in the presence of various amounts of near field hydrogen are presented. Studies of the dissolution of 233 U doped UO 2 (s) simulating 'old' spent fuel were carried out as static leaching tests, autoclave tests with various hydrogen concentrations and electrochemical tests. The results of the leaching behaviour of a high burn-up spent fuel pellet in 5 M NaCl solutions in the presence of 3.2 bar H 2 pressure and of MOX fuel in dilute synthetic groundwater under 53 bar H 2 pressure are also presented. In all the experimental studies carried out in this project, a considerable effect of hydrogen in the dissolution rates of radioactive materials was observed. The experimental results obtained in this project with a-doped UO 2 , high burn-up spent fuel and MOX fuel together with literature data give a reliable background to use fractional alteration/dissolution rates for spent fuel of the order of 10 -6 /yr - 10 -8 /yr with a recommended value of 4x10 -7 /yr for dissolved hydrogen concentrations above 10 -3 M and Fe(II) concentrations typical for European repository concepts. Finally, based on a review of the experimental data and available literature data, potential mechanisms of the hydrogen effect are also discussed. The work reported in this document was performed as part of the Project SFS of the European Commission 5th Framework Programme under contract no FIKW-CT-2001-20192 SFS. It represents the deliverable D10 of the experimental work package 'Key experiments using a-doped UO 2 and real spent fuel', coordinated by SKB with the participation of ITU, FZK-INE, ENRESA, CIEMAT, ARMINES-SUBATECH and SKB

MOX fuel irradiation behaviour: Results from X-ray microbeam analysis

International Nuclear Information System (INIS)

Walker, C.T.; Goll, W.; Matsumura, T.

1997-01-01

The behaviour of plutonium, xenon and caesium were investigated in two sections of irradiated MOX fuel produced by the OCOM process. In one fuel (OCOM30), the MOX agglomerates contained 18 wt% fissile plutonium, and had a low volume fraction of 0.17; in the other (OCOM15) the agglomerates contained 9 wt% fissile plutonium, and had a high volume fraction of 0.34. Both fuels had been irradiated under normal power reactor conditions to a burn-up of approximately 44 GWd/t. The main aim of the work was to establish whether the above differences in composition affected the percentage fission gas released by the fuels. Since U/Pu interdiffusion did not occurred during the irradiation, both fuels remained inhomogeneous on the microscopic scale. However, the concentration of plutonium in the MOX agglomerates decreases by about 50% as a result of fission, whereas the plutonium content of the UO 2 matrix increased by about a factor of four to approximately 2 wt% due to neutron capture by 238 U. The agglomerates in the OCOM15 fuel generally exhibited a finer structure due to the lower burn-up. More than 80% of the fission gas had been released from the oxide lattice of the MOX agglomerates in both fuels. However, a very high fraction of this gas precipitated and remained in the pore structure of the agglomerates. Consequently, puncturing revealed that for both fuels the percentage of gas released to the rod free volume increased from less than 0.5% at 10 GWd/t to a maximum of 3.5% at 45 GWd/t. The conclusion is that the percentage of gas released by MOX fuel is largely unaffected of the level of inhomogeneity of the fuel. In both fuels caesium showed near complete retention in both the MOX agglomerates and the UO 2 matrix. (author). 8 refs, 11 figs, 3 tabs

Parametric studies of the effect of MOx environment and control rods for PWR-UOx burnup credit implementation

International Nuclear Information System (INIS)

Barreau, Anne; Roque, Benedicte; Marimbeau, Pierre; Venard, Christophe; Bioux, Philippe; Toubon, Herve

2003-01-01

The increase of PWR-UOX fuel initial enrichment and the extensive needs for spent fuel storage or cask capacities reinforce the interest in taking burnup credit into account in criticality calculations. However, this utilization of credit for fuel burnup requires the definition of a methodology that ensures the conservatism of calculations. In order to guarantee the conservatism of the spent fuel inventory calculation, a depletion calculation scheme for burnup credit is under development. This paper presents the studies on the main parameters which have an effect on nuclides concentration: the presence of control rods during depletion and the fuel assembly environment, particularly the presence of MOx fuels around the UO 2 assembly. Reactivity effects which are relevant to these parameters are then presented, and physics phenomena are identified. (author)

Isotopic analyses and calculation by use of JENDL-3.2 for high burn-up UO{sub 2} and MOX spent fuels

Energy Technology Data Exchange (ETDEWEB)

Sasahara, Akihiro; Matsumura, Tetsuo [Central Research Inst. of Electric Power Industry, Komae, Tokyo (Japan). Komae Research Lab.; Nicolaou, G.; Betti, M.; Walker, C.T.

1997-03-01

The post irradiation examinations (PIE) were carried out for high burn-up UO{sub 2} spent fuel (3.8%U235, average burn-up:60GWd/t) and mixed oxide (MOX) spent fuel (5.07%Pu, average burn-up:45GWd/t). The PIE includes, (a) isotopic analysis, (b) electron probe microanalysis (EPMA) in pellet cross section and so on. The results of isotopic analyses and EPMA were compared with ORIGEN2/82 and VIM-BURN calculation results. In VIM-BURN calculation, the nuclear data of actinides were proceeded from new data file, JENDL-3.2. The sensitivities of power history and moderator density to nuclides composition were investigated by VIM-BURN calculation and consequently power history mainly effected on Am241 and Am242m and moderator density effected on fissile nuclides. From EPMA results of U and Pu distribution in pellet, VIM-BURN calculation showed reasonable distribution in pellet cross section. (author)

MOX - equilibrium core design and trial irradiation in KAPS - 1

International Nuclear Information System (INIS)

Pradhan, A.S.; Ray, Sherly; Kumar, A.N.; Parikh, M.V.

2006-01-01

Option of usage of MOX fuel bundles in the equilibrium core of Indian 220 MWe PHWRs on a regular basis has been studied. The design of the MOX bundle considered is MOX -7 with inner 7 elements with uranium and plutonium oxide MOX fuel and outer 12 elements with natural uranium fuel. The composition of the plutonium isotopes corresponds to that at about 6500 MWD/TeU burnup. Burnup optimization has been done such that operation at design rated power is possible while achieving the maximum average discharge burnup. Operation with the optimized burnup pattern will result in substantial saving of natural uranium bundles. To obtain feedback on the performance of MOX bundles prior to its large scale use about 50 MOX-7 bundles have been loaded in KAPS - 1 equilibrium core. Locations have been selected such that reactor should be operating at rated power without violating any constraints on channel bundle powers and also meeting the safety requirements. Burnup of interest also should be achieved in minimum period of time. The fissile plutonium content in the 50 MOX fuel bundles loaded is about 75.6 wt % . About 38 bundles out of the 50 bundles loaded have been already discharged and remaining bundles are still in the core. The maximum discharge burnup of the MOX bundles is about 12000 MWD/TeU. The performance of the MOX bundles were excellent and as per prediction. No MOX bundle is reported to be failed. (author)

High burn-up structure in nuclear fuel: impact on fuel behavior - 4005

International Nuclear Information System (INIS)

Noirot, J.; Pontillon, Y.; Zacharie-Aubrun, I.; Hanifi, K.; Bienvenu, P.; Lamontagne, J.; Desgranges, L.

2016-01-01

When UO 2 and (U,Pu)O 2 fuels locally reach high burn-up, a major change in the microstructure takes place. The initial grains are replaced by thousands of much smaller grains, fission gases form micrometric bubbles and metallic fission products form precipitates. This occurs typically at the rim of the pellets and in heterogeneous MOX fuel Pu rich agglomerates. The high burn-up at the rim of the pellets is due to a high capture of epithermal neutrons by 238 U leading locally to a higher concentration of fissile Pu than in the rest of the pellet. In the heterogeneous MOX fuels, this rim effect is also active, but most of the high burn-up structure (HBS) formation is linked to the high local concentration of fissile Pu in the Pu agglomerates. This Pu distribution leads to sharp borders between HBS and non-HBS areas. It has been shown that the size of the new grains, of the bubbles and of the precipitates increase with the irradiation local temperatures. Other parameters have been shown to have an influence on the HBS initiation threshold, such as the irradiation density rate, the fuel composition with an effect of the Pu presence, but also of the Gd concentration in poisoned fuels, some of the studied additives, like Cr, and, maybe some of the impurities. It has been shown by indirect and direct approaches that HBS formation is not the main contributor to the increase of fission gas release at high burn-up and that the HBS areas are not the main source of the released gases. The impact of HBS on the fuel behavior during ramp on high burn-up fuels is still unclear. This short paper is followed by the slides of the presentation

Present status of reactor physics in the United States and Japan-IV. 2. Micro-Reactor Physics of MOX-Fueled Core

International Nuclear Information System (INIS)

Takeda, Toshikazu

2001-01-01

Recently, fuel assemblies of light water reactors have become complicated because of the extension of fuel burnup and the use of high-enriched Gd and mixed-oxide (MOX) fuel, etc. In conventional assembly calculations, the detailed flux distribution, spectrum distribution, and space dependence of self-shielding within a fuel pellet are not directly taken into account. The experimental and theoretical study of investigating these microscopic properties is named micro-reactor physics. The purpose of this work is to show the importance of micro-reactor physics in the analysis of MOX fuel assemblies. Several authors have done related studies; however, their studies are limited to fuel pin cells, and they are never mentioned with regard to burnup effect, which is important for actual core design. We used the subgroup method to treat the space dependence of the self-shielding effect of heavy nuclides, and we used the characteristics method to treat the angular dependence of neutron flux in a fuel pellet. Figure 1 compares the power distributions in MOX and UO 2 fuel cells at the beginning of burnup. The power is calculated with and without considering the space dependence of the self-shielding effect of the cross sections. For the MOX cell, the power distribution has a peak at the cell edge because of large Pu absorption especially when considering the spatial self-shielding effect. When a MOX rod is adjacent to UO 2 fuel rods, the flux distribution has an azimuthal dependence in addition to the radial dependence within a rod. For example, consider a 2x2 fuel assembly composed of three UO 2 rods and one MOX rod, with the mirror reflection boundary condition. A burnup calculation was done with the condition; the radius of the MOX pellet is divided into two regions, and the azimuthal angle is divided into eight. The number density of 239 Pu at 44 000 MWd/t for the MOX rod shows azimuthal dependence by 20%. The maximum burnup occurs in the direction of the UO 2 rods. This is

Analysis of Radial Plutonium Isotope Distribution in Irradiated Test MOX Fuel Rods

Energy Technology Data Exchange (ETDEWEB)

Oh, Jae Yong; Lee, Byung Ho; Koo, Yang Hyun; Kim, Han Soo

2009-01-15

After Rod 3 and 6 (KAERI MOX) were irradiated in the Halden reactor, their post-irradiation examinations are being carried out now. In this report, PLUTON code was implemented to analyze Rod 3 and 6 (KAERI MOX). In the both rods, the ratio of a maximum burnup to an average burnup in the radial distribution was 1.3 and the contents of {sup 239}Pu tended to increase as the radial position approached the periphery of the fuel pellet. The detailed radial distribution of {sup 239}Pu and {sup 240}Pu, however, were somewhat different. To find the reason for this difference, the contents of Pu isotopes were investigated as the burnup increased. The content of {sup 239}Pu decreased with the burnup. The content of {sup 240}Pu increased with the burnup by the 20 GWd/tM but decreased over the 20 GWd/tM. The local burnup of Rod 3 is higher than that of Rod 6 due to the hole penetrated through the fuel rod. The content of {sup 239}Pu decreased more rapidly than that of {sup 240}Pu in the Rod 6 with the increased burnup. It resulted in a radial distribution of {sup 239}Pu and {sup 240}Pu similar to Rod 3. The ratio of Xe to Kr is a parameter to find where the fissions occur in the nuclear fuel. In both Rod 3 and 6, it was 18.3 in the whole fuel rod cross section, which showed that the fissions occurred in the plutonium.

An overview of economic and technical issues related to LWR MOX fuel usage

International Nuclear Information System (INIS)

Malone, J.P.; Varley, G.; Goldstein, L.

1999-01-01

This paper will present comparisons of the economics of MOX versus UO 2 fuels. In addition to the economics of the front end, the scope of the comparison will include the back end of the fuel cycle. Management of spent MOX fuel assemblies presents utilities with some technical issues that can complicate spent fuel pool operation. Alternative spent fuel management methods, such as dry storage of spent MOX fuel assemblies, will also be discussed. Differences in decay heat loads versus time for spent MOX and UO 2 fuel assemblies will be presented. This difference is one of the main problems confronting spent fuel managers relative to MOX. The difference in decay heat loads will serve as the basis for a performance overview of the various spent fuel technologies available today. The economics of the front end of MOX will be presented relative to UO 2 fuel. Availability of MOX manufacturing capability will also be discussed, along with a discussion of its impact on future MOX fabrication prices. The in-core performance of MOX will be compared to that of UO 2 fuel with similar performance characteristics. The information will include highlights of nuclear design and related operational considerations such as: Reactivity reduction with burnup is slower for MOX fuel than for UO 2 fuel; Spectral hardening resulting in lower control rod worths and a lower soluble boron worth; and more negative moderator, void and fuel temperature coefficients. A comparison of Westinghouse and ABB-CE core designs for use on disposition of weapons MOX in 12- and 18-month cycles will be presented. (author)

MOX fuel cycle technologies for medium and long term deployment. Proceedings

Energy Technology Data Exchange (ETDEWEB)

NONE

2000-07-01

More than thirty years of reactor experience using MOX fuel as well as the fabrication of 2000 MOX assemblies with the use of 85 t of Pu separated from spent fuel from power reactors indicates that the recycling of plutonium as MOX fuel in LWRs has become a mature industry. The number of countries engaged in plutonium recycling could be increasing in the near future, aiming for the reduction of stockpiles of separated plutonium from earlier and existing reprocessing contracts. Economic and strategic considerations are the main factors on which to base such a decision to use MOX. Transport of MOX fuel assemblies is a vital element in these recycle programmes but could have the potential to be a weak link in the chain. To avoid problems, it is essential that sufficient numbers of transport flasks of the required types, licensed for the increasing Pu contents, be made available in a timely manner to keep pace with the planned increases in fabrication rates. Despite the excellent safety records for radioactive and MOX transports over many decades, continuous attention should be drawn to establishing the transport modalities, buffer stores, secure vehicles, and transport routes, at the same time accounting for public sensitivities on radioactive transports in general and MOX transport in particular. A large number of technical presentations updated and reconfirmed the good and almost defect-free performance of MOX fuel at increasingly high burn-up levels. MOX fuel is designed to meet the same operational and safety criteria as uranium fuels under equivalent conditions. This is also confirmed by the parallel development of design codes to accommodate the special characteristics of MOX. Integral and specific parameter testing of MOX fuel in normal and off-normal operation is under way in a number of countries with particular emphasis on high burnup behaviour. Here the important contributions of the OECD/NEA Halden BWR programme should be mentioned. The reactor

MOX fuel cycle technologies for medium and long term deployment. Proceedings

International Nuclear Information System (INIS)

2000-01-01

More than thirty years of reactor experience using MOX fuel as well as the fabrication of 2000 MOX assemblies with the use of 85 t of Pu separated from spent fuel from power reactors indicates that the recycling of plutonium as MOX fuel in LWRs has become a mature industry. The number of countries engaged in plutonium recycling could be increasing in the near future, aiming for the reduction of stockpiles of separated plutonium from earlier and existing reprocessing contracts. Economic and strategic considerations are the main factors on which to base such a decision to use MOX. Transport of MOX fuel assemblies is a vital element in these recycle programmes but could have the potential to be a weak link in the chain. To avoid problems, it is essential that sufficient numbers of transport flasks of the required types, licensed for the increasing Pu contents, be made available in a timely manner to keep pace with the planned increases in fabrication rates. Despite the excellent safety records for radioactive and MOX transports over many decades, continuous attention should be drawn to establishing the transport modalities, buffer stores, secure vehicles, and transport routes, at the same time accounting for public sensitivities on radioactive transports in general and MOX transport in particular. A large number of technical presentations updated and reconfirmed the good and almost defect-free performance of MOX fuel at increasingly high burn-up levels. MOX fuel is designed to meet the same operational and safety criteria as uranium fuels under equivalent conditions. This is also confirmed by the parallel development of design codes to accommodate the special characteristics of MOX. Integral and specific parameter testing of MOX fuel in normal and off-normal operation is under way in a number of countries with particular emphasis on high burnup behaviour. Here the important contributions of the OECD/NEA Halden BWR programme should be mentioned. The reactor

MOX fuel fabrication technology in J-MOX

International Nuclear Information System (INIS)

Osaka, Shuichi; Yoshida, Ryouichi; Yamazaki, Yukiko; Ikeda, Hiroyuki

2014-01-01

Japan Nuclear Fuel Ltd. (JNFL) has constructed JNFL MOX Fuel Fabrication Plant (J-MOX) since 2010. The MIMAS process has been introduced in the powder mixing process from AREVA NC considering a lot of MOX fuel fabrication experiences at MELOX plant in France. The feed material of Pu for J-MOX is MH-MOX powder from Rokkasho Reprocessing Plant (RRP) in Japan. The compatibility of the MH-MOX powder with the MIMAS process was positively evaluated and confirmed in our previous study. This paper describes the influences of the UO2 powder and the recycled scrap powder on the MOX pellet density. (author)

Investigation of research and development subjects for the Very High Burnup Fuel

International Nuclear Information System (INIS)

Hayashi, Kimio; Amano, Hidetoshi; Suzuki, Yasufumi; Furuta, Teruo; Nagase, Fumihisa; Suzuki, Masahide

1993-06-01

A concept of the Very High Burnup Fuel aiming at a maximum fuel assembly burnup of 100 GWd/t has been proposed in terms of burnup extension, utilization of Pu and transmutation of transuranium elements (TRU: Np, Am and Cm). The authors have investigated research and development (R and D) subjects of the fuel pellet and the cladding material of the Fuel. The present report describes the results on the fuel pellet. First, the chemical state of the Fuel and fission products (FP) was inferred through an FP-inventory and an equilibrium-thermodynamics calculations. Besides, knowledge obtained from post-irradiation examinations was surveyed. Next, an investigation was made on irradiation behavior of U/Pu mixed oxide (MOX) fuel with high enrichment of Pu, as well as on fission-gas release and swelling behavior of high burnup fuels. Reprocessibility of the Fuel, particularly solubility of the spent fuel, was also examined. As for the TRU-added fuel, material property data on TRU oxides were surveyed and summarized as a database. And the subjects on the production and the irradiation behavior were examined on the basis of experiences of MOX fuel production and TRU-added fuel irradiation. As a whole, the present study revealed the necessity of accumulating fundamental data and knowledge required for design and assessment of the fuel pellet, including the information on properties and irradiation performance of the TRU-added fuel. Finally, the R and D subjects were summarized, and a proposal was made on the way of development of the fuel pellet and cladding materials. (author)

Fuel rod design by statistical methods for MOX fuel

International Nuclear Information System (INIS)

Heins, L.; Landskron, H.

2000-01-01

Statistical methods in fuel rod design have received more and more attention during the last years. One of different possible ways to use statistical methods in fuel rod design can be described as follows: Monte Carlo calculations are performed using the fuel rod code CARO. For each run with CARO, the set of input data is modified: parameters describing the design of the fuel rod (geometrical data, density etc.) and modeling parameters are randomly selected according to their individual distributions. Power histories are varied systematically in a way that each power history of the relevant core management calculation is represented in the Monte Carlo calculations with equal frequency. The frequency distributions of the results as rod internal pressure and cladding strain which are generated by the Monte Carlo calculation are evaluated and compared with the design criteria. Up to now, this methodology has been applied to licensing calculations for PWRs and BWRs, UO 2 and MOX fuel, in 3 countries. Especially for the insertion of MOX fuel resulting in power histories with relatively high linear heat generation rates at higher burnup, the statistical methodology is an appropriate approach to demonstrate the compliance of licensing requirements. (author)

Taking burnup credit for interim storage and transportation system for BWR fuels

International Nuclear Information System (INIS)

Yoshioka, Ken-ichi; Ando, Y.; Kumanomido, H.; Sasaki, T.; Mitsuhashi, I.; Ueda, M.

2001-01-01

In order to establish a realistic burnup credit design system, a calculation system has been developed for determining isotope compositions, burnup, and criticality. The calculation system consists of several modules such as TGBLA, ORIGEN, CITATION, MCNP, and KENO. The TGBLA code is a fuel design code for LWR fuels developed in TOSHIBA Corporation. A compact measurement system for a fuel assembly has been being developed to meet requirements for the burnup determination, the neutron emission-rate evaluation, and the nuclear materials management. For a spent MOX fuel, a neutron emission rate measurement method has been being developed. The system consists of Cd-Te detectors and / or fission chambers. Some model calculations were carried out for the latest design BWR fuels. The effect of taking burnup credit for a transportation cask is shown. (authors)

The effect of dissolved hydrogen on the dissolution of {sup 233}U doped UO{sub 2}(s) high burn-up spent fuel and MOX fuel

Energy Technology Data Exchange (ETDEWEB)

Carbol, P. [Inst. for Transuranium Elements, Karlsruhe (Germany); Spahiu, K. (ed.) [and others

2005-03-01

In this report the results of the experimental work carried out in a large EU-research project (SFS, 2001-2004) on spent fuel stability in the presence of various amounts of near field hydrogen are presented. Studies of the dissolution of {sup 233}U doped UO{sub 2}(s) simulating 'old' spent fuel were carried out as static leaching tests, autoclave tests with various hydrogen concentrations and electrochemical tests. The results of the leaching behaviour of a high burn-up spent fuel pellet in 5 M NaCl solutions in the presence of 3.2 bar H{sub 2} pressure and of MOX fuel in dilute synthetic groundwater under 53 bar H{sub 2} pressure are also presented. In all the experimental studies carried out in this project, a considerable effect of hydrogen in the dissolution rates of radioactive materials was observed. The experimental results obtained in this project with a-doped UO{sub 2}, high burn-up spent fuel and MOX fuel together with literature data give a reliable background to use fractional alteration/dissolution rates for spent fuel of the order of 10{sup -6}/yr - 10{sup -8}/yr with a recommended value of 4x10{sup -7}/yr for dissolved hydrogen concentrations above 10{sup -3} M and Fe(II) concentrations typical for European repository concepts. Finally, based on a review of the experimental data and available literature data, potential mechanisms of the hydrogen effect are also discussed. The work reported in this document was performed as part of the Project SFS of the European Commission 5th Framework Programme under contract no FIKW-CT-2001-20192 SFS. It represents the deliverable D10 of the experimental work package 'Key experiments using a-doped UO{sub 2} and real spent fuel', coordinated by SKB with the participation of ITU, FZK-INE, ENRESA, CIEMAT, ARMINES-SUBATECH and SKB.

The effect of dissolved hydrogen on the dissolution of {sup 233}U doped UO{sub 2}(s) high burn-up spent fuel and MOX fuel

Energy Technology Data Exchange (ETDEWEB)

Carbol, P [Inst. for Transuranium Elements, Karlsruhe (Germany); Spahiu, K [and others

2005-03-01

In this report the results of the experimental work carried out in a large EU-research project (SFS, 2001-2004) on spent fuel stability in the presence of various amounts of near field hydrogen are presented. Studies of the dissolution of {sup 233}U doped UO{sub 2}(s) simulating 'old' spent fuel were carried out as static leaching tests, autoclave tests with various hydrogen concentrations and electrochemical tests. The results of the leaching behaviour of a high burn-up spent fuel pellet in 5 M NaCl solutions in the presence of 3.2 bar H{sub 2} pressure and of MOX fuel in dilute synthetic groundwater under 53 bar H{sub 2} pressure are also presented. In all the experimental studies carried out in this project, a considerable effect of hydrogen in the dissolution rates of radioactive materials was observed. The experimental results obtained in this project with a-doped UO{sub 2}, high burn-up spent fuel and MOX fuel together with literature data give a reliable background to use fractional alteration/dissolution rates for spent fuel of the order of 10{sup -6}/yr - 10{sup -8}/yr with a recommended value of 4x10{sup -7}/yr for dissolved hydrogen concentrations above 10{sup -3} M and Fe(II) concentrations typical for European repository concepts. Finally, based on a review of the experimental data and available literature data, potential mechanisms of the hydrogen effect are also discussed. The work reported in this document was performed as part of the Project SFS of the European Commission 5th Framework Programme under contract no FIKW-CT-2001-20192 SFS. It represents the deliverable D10 of the experimental work package 'Key experiments using a-doped UO{sub 2} and real spent fuel', coordinated by SKB with the participation of ITU, FZK-INE, ENRESA, CIEMAT, ARMINES-SUBATECH and SKB.

Radial power density distribution of MOX fuel rods in the IFA-651

Energy Technology Data Exchange (ETDEWEB)

Lee, Byung Ho; Koo, Yang Hyun; Joo, Hyung Kook; Cheon, Jin Sik; Oh, Je Yong; Sohn, Dong Seong [Korea Atomic Energy Research Institute, Taejeon (Korea)

2002-04-01

Two MOX fuel rods, which were fabricated in the Paul Scherrer Institute (PSI), Switzerland in cooperation with Korea Atomic Energy Research Institute, have been irradiated in the HBWR from June, 2000 in the framework of OECD-HRP together with a reference MOX fuel rod supplied by the BNFL. Since fuel temperature, which is influenced by radial power distribution, is basic in analyzing fuel behavior, it is required to consider radial power distribution in the HBWR. A subroutine FACTOR{sub H}BWR that calculates radial power density distribution for three MOX fuel rods has been developed based on neutron physics results and DEPRESS program. The developed subroutine FACTOR{sub H}BWR gives good agreement with the physics calculation except slight under-prediction at the outer part of the pellet above the burnup of 20 MWd/kgHM. The subroutine will be incorporated into a computer code COSMOS and used to analyze the in-reactor behavior of the three MOX fuel rods during the Halden irradiation test. 24 figs., 4 tabs. (Author)

The MOX fuel behaviour test IFA-597.4/.5/.6/.7; Summary of in-pile fuel temperature and gas release data

Energy Technology Data Exchange (ETDEWEB)

Koike, Hisashi

2003-11-15

It is considered important to study the in-reactor behaviour of MOX fuel in order to enhance the database on such fuel. For this reason, IFA-597.4/.5/.6/.7 were included in the joint research programme of the Halden Project. The series of tests, containing two MIMAS-MOX fuel rods, both equipped with a fuel centre thermocouple and a pressure bellows transducer, has been irradiated in the Halden Reactor since July 1997 under HBWR conditions. The objectives of the test series were to study the thermal and fission gas release (FGR) behaviour of MOX fuel and to explore potential differences in behaviour between solid and hollow pellets. One of the rods had mainly solid pellets, while the other contained only hollow pellets. Both rods had an initial Pu-fissile enrichment of 6.07%. The cladding outside diameter was 9.50 mm, and the initial fuel-clad gap was 180 mum. In the course of the test, power upratings for FGR studies of the MOX fuel were planned at burnup intervals of about 10 MWd/kg MOX. The power uprating was successfully performed at approx10 MWd/kg MOX, where the estimated fuel peak temperature of the solid pellets exceeded the FGR threshold temperature for UO{sub 2} fuel, while that of the hollow pellets remained below the threshold. For the solid fuel, the temperature at onset of FGR was consistent with the empirical threshold temperature for UO{sub 2} fuel. For the hollow fuel, gas release was observed at temperatures below the threshold. FGRs at the end-of-life were approx17% for the solid pellet rod and approx14% for the hollow pellet rod, respectively. As a result of discussions in HPG meetings, IFA-597.7 was unloaded in January 2002. PIE was carried out to check in-pile pressure measurements and examine fuel structural characteristics. The discharge burn-up of the MOX fuel was 32 MWd/kg MOX as determined from in-pile power data. This report supersedes HWR-712 (June 2002) previously issued on in-pile data from IFA-597.4/5/6/7. (Author)

Developments in MOX fuel pellet fabrication technology: Indian experience

International Nuclear Information System (INIS)

Kamath, H.S.; Majumdar, S.; Purusthotham, D.S.C.

1998-01-01

India is interested in mixed oxide (MOX) fuel technology for better utilisation of its nuclear fuel resources. In view of this, a programme involving MOX fuel design, fabrication and irradiation in research and power reactors has been taken up. A number of experimental irradiations in research reactors have been carried out and a few MOX assemblies of ''All Pu'' type have been loaded in our commercial BWRs at Tarapur. An island type of MOX fuel design is under study for use in PHWRs which can increase the burn-up of the fuel by more than 30% compared to natural UO 2 fuel. The MOX fuel pellet fabrication technology for the above purpose and R and D efforts in progress for achieving better fuel performance are described in the paper. The standard MOX fuel fabrication route involves mechanical mixing and milling of UO 2 and PuO 2 powders. After detailed investigations with several types of mixing and milling equipments, dry attritor milling has been found to be the most suitable for this operation. Neutron Coincident Counting (NCC) technique was found to be the most convenient and appropriate technique for quick analysis of Pu content in milled MOX powder and to know Pu mixing is homogenous or not. Both mechanical and hydraulic presses have been used for powder compaction for green pellet production although the latter has been preferred for better reproducibility. Low residue admixed lubricants have been used to facilitate easy compaction. The normal sintering temperature used in Nitrogen-Hydrogen atmosphere is between 1600 deg. C to 1700 deg. C. Low temperature sintering (LTS) using oxidative atmospheres such as carbon dioxide, Nitrogen and coarse vacuum have also been investigated on UO 2 and MOX on experimental scale and irradiation behaviour of such MOX pellets is under study. Ceramic fibre lined batch furnaces have been found to be the most suitable for MOX pellet production as they offer very good flexibility in sintering cycle, and ease of maintainability

MOX fuel reprocessing and recycling

International Nuclear Information System (INIS)

Guillet, J.L.

1990-01-01

This paper is devoted to the reprocessing of MOX fuel in UP2-800 plant at La Hague, and to the MOX successive reprocessing and recycling. 1. MOX fuel reprocessing. In a first step, the necessary modifications in UP2-800 to reprocess MOX fuel are set out. Early in the UP2-800 project, actions have been taken to reprocess MOX fuel without penalty. They consist in measures regarding: Dissolution; Radiological shieldings; Nuclear instrumentation; Criticality. 2. Mox successive reprocessing and recycling. The plutonium recycling in the LWR is now a reality and, as said before, the MOX fuel reprocessing is possible in UP2-800 plant at La Hague. The following actions in this field consist in verifying the MOX successive reprocessing and recycling possibilities. After irradiation, the fissile plutonium content of irradiated MOX fuel is decreased and, in this case, the re-use of plutonium in the LWR need an important increase of initial Pu enrichment inconsistent with the Safety reactor constraints. Cogema opted for reprocessing irradiated MOX fuel in dilution with the standard UO2 fuel in appropriate proportions (1 MOX for 4 UO2 fuel for instance) in order to save a fissile plutonium content compatible with MOX successive recycling (at least 3 recyclings) in LWR. (author). 2 figs

MOX Cross-Section Libraries for ORIGEN-ARP

International Nuclear Information System (INIS)

Gauld, I.C.

2003-01-01

The use of mixed-oxide (MOX) fuel in commercial nuclear power reactors operated in Europe has expanded rapidly over the past decade. The predicted characteristics of MOX fuel such as the nuclide inventories, thermal power from decay heat, and radiation sources are required for design and safety evaluations, and can provide valuable information for non-destructive safeguards verification activities. This report describes the development of computational methods and cross-section libraries suitable for the analysis of irradiated MOX fuel with the widely-used and recognized ORIGEN-ARP isotope generation and depletion code of the SCALE (Standardized Computer Analyses for Licensing Evaluation) code system. The MOX libraries are designed to be used with the Automatic Rapid Processing (ARP) module of SCALE that interpolates appropriate values of the cross sections from a database of parameterized cross-section libraries to create a problem-dependent library for the burnup analysis. The methods in ORIGEN-ARP, originally designed for uranium-based fuels only, have been significantly upgraded to handle the larger number of interpolation parameters associated with MOX fuels. The new methods have been incorporated in a new version of the ARP code that can generate libraries for low-enriched uranium (LEU) and MOX fuel types. The MOX data libraries and interpolation algorithms in ORIGEN-ARP have been verified using a database of declared isotopic concentrations for 1042 European MOX fuel assemblies. The methods and data are validated using a numerical MOX fuel benchmark established by the Organization for Economic Cooperation and Development (OECD) Working Group on burnup credit and nuclide assay measurements for irradiated MOX fuel performed as part of the Belgonucleaire ARIANE International Program

Mox fuels recycling

International Nuclear Information System (INIS)

Gay, A.

1998-01-01

This paper will firstly emphasis that the first recycling of plutonium is already an industrial reality in France thanks to the high degree of performance of La Hague and MELOX COGEMA's plants. Secondly, recycling of spent Mixed OXide fuel, as a complete MOX fuel cycle, will be demonstrated through the ability of the existing plants and services which have been designed to proceed with such fuels. Each step of the MOX fuel cycle concept will be presented: transportation, reception and storage at La Hague and steps of spent MOX fuel reprocessing. (author)

Nuclear fuel behaviour modelling at high burnup and its experimental support. Proceedings of a technical committee meeting

International Nuclear Information System (INIS)

2001-07-01

The Technical Committee Meeting (TCM) included separate sessions on the specific topics of fuel thermal performance and fission product retention. On thermal performance, it is apparent that the capability exists to measure conductivity in high burnup fuel either by out-of-pile measurement or by instrumentation of test reactor rods. State-of-the-art modelling codes contain models for the conductivity degradation process, and hence adequate predictions of fuel temperature are achievable. Concerning fission product release, it is clear that many groups around the world are actively investigating the subject, with experimental and modelling programmes being pursued. However, a general consensus on the exact mechanisms of gas release and related gas bubble swelling has yet to emerge, even at medium burnup levels. Fission gas phenomena, not only the release to open volumes, but the whole sequence of processes taking place prior to this, need to be modelled in any modern fuel performance code. The presence of gaseous fission products may generate rapid fuel swelling during power transients, and this can cause PCI and rod failure. At high burnups, the quantity of released gases could give rise to pressures exceeding the safe limits. Modelling of pellet-cladding interaction (PCI) effects during transient operation is also an active area of study for many groups. In some situations a purely empirical approach to failure modelling can be justified, while for other applications a more detailed mechanistic approach is required. Another aspect of cladding modelling which was featured at the TCM concerned corrosion and hydriding. Although this issue can be the main life-limiting factor on fuel duty, it is apparent that modelling methods, and the experimental measurement techniques that underpin them, are adequate. A session was included on MOX fuel modelling. Substantial programmes of work, especially by the MOX vendors, appear to be underway to bring the level of understanding

A utility analysis of MOX recycling policy

International Nuclear Information System (INIS)

Pfaeffli, J.L.

1990-01-01

The author presents the advantages of recycling of plutonium and uranium from spent reactor fuel assemblies as follows: natural uranium and enrichment savings, mixed oxide fuel (MOX) fuel assembly cost, MOX compatibility with plant operation, high burnups, spent MOX reprocessing, and non-proliferation aspects.Disadvantages of the recycling effort are noted as well: plutonium degradation with time, plutonium availability, in-core fuel management, administrative authorizations by the licensings authorities, US prior consent, and MOX fuel fabrication capacity. Putting the advantages and disadvantages in perspective, it is concluded that the recycling of MOX in light water reactors represents, under the current circumstances, the most appropriate way of making use of the available plutonium

The transportation of PuO2 and MOX fuel and management of irradiated MOX fuel

International Nuclear Information System (INIS)

Dyck, H.P.; Rawl, R.; Durpel, L. van den

2000-01-01

Information is given on the transportation of PuO 2 and mixed-oxide (MOX) fuel, the regulatory requirements for transportation, the packages used and the security provisions for transports. The experience with and management of irradiated MOX fuel and the reprocessing of MOX fuel are described. Information on the amount of MOX fuel irradiated is provided. (author)

Results of Am isotopic ratio analysis in irradiated MOX fuels

Energy Technology Data Exchange (ETDEWEB)

Koyama, Shin-ichi; Osaka, Masahiko; Mitsugashira, Toshiaki; Konno, Koichi [Power Reactor and Nuclear Fuel Development Corp., Oarai, Ibaraki (Japan). Oarai Engineering Center; Kajitani, Mikio

1997-04-01

For analysis of a small quantity of americium, it is necessary to separate from curium which has similar chemical property. As a chemical separation method for americium and curium, the oxidation of americium with pentavalent bismuth and subsequent co-precipitation of trivalent curium with BIP O{sub 4} were applied to analyze americium in irradiated MOX fuels which contained about 30wt% plutonium and 0.9wt% {sup 241}Am before irradiation and were irradiated up to 26.2GWd/t in the experimental fast reactor Joyo. The purpose of this study is to measure isotopic ratio of americium and to evaluate the change of isotopic ratio with irradiation. Following results are obtained in this study. (1) The isotopic ratio of americium ({sup 241}Am, {sup 242m}Am and {sup 243}Am) can be analyzed in the MOX fuels by isolating americium. The isotopic ratio of {sup 242m}Am and {sup 243}Am increases up to 0.62at% and 0.82at% at maximum burnup, respectively, (2) The results of isotopic analysis indicates that the contents of {sup 241}Am decreases, whereas {sup 242m}Am, {sup 243}Am increase linearly with increasing burnup. (author)

Plant overview of JNFL MOX fuel fabrication plant (J-MOX)

International Nuclear Information System (INIS)

Hiruta, Kazuhiko; Suzuki, Masataka; Shimizu, Junji; Suzuki, Kazumi; Yamamoto, Yutaka; Deguchi, Morimoto; Fujimaki, Kazunori

2005-01-01

In April 2005, JNFL submitted METI an application for the permission of MOX fuel fabrication business for JNFL MOX Fuel Fabrication Plant (J-MOX). Accordingly, safeguards formalities and discussion with the Agency have been also started for J-MOX as an official project. This report describes J-MOX plant overview and also presents outline of J-MOX by focusing on safeguards features and planned material accountancy method. (author)

Calculation of pellet radial power distributions with a Monte Carlo burnup code

International Nuclear Information System (INIS)

Suzuki, Motomu; Yamamoto, Toru; Nakata, Tetsuo

2010-01-01

The Japan Nuclear Energy Safety Organization (JNES) has been working on an irradiation test program of high-burnup MOX fuel at Halden Boiling Water Reactor (HBWR). MOX and UO 2 fuel rods had been irradiated up to about 64 GWd/t (rod avg.) as a Japanese utilities research program (1st phase), and using those fuel rods, in-situ measurement of fuel pellet centerline temperature was done during the 2nd phase of irradiation as the JNES test program. As part of analysis of the temperature data, power distributions in a pellet radial direction were analyzed by using a Monte Carlo burnup code MVP-BURN. In addition, the calculated results of deterministic burnup codes SRAC and PLUTON for the same problem were compared with those of MVP-BURN to evaluate their accuracy. Burnup calculations with an assembly model were performed by using MVP-BURN and those with a pin cell model by using SRAC and PLUTON. The cell pitch and, therefore, fuel to moderator ratio in the pin cell calculation was determined from the comparison of neutron energy spectra with those of MVP-BURN. The fuel pellet radial distributions of burnup and fission reaction rates at the end of the 1st phase irradiation were compared between the three codes. The MVP-BURN calculation results show a large peaking in the burnup and fission rates in the pellet outer region for the UO 2 and MOX pellets. The SRAC calculations give very close results to those of the MVP-BURN. On the other hand, the PLUTON calculations show larger burnup for the UO 2 and lower burnup for the MOX pellets in the pellet outer region than those of MVP-BURN, which lead to larger fission rates for the UO 2 and lower fission rates for the MOX pellets, respectively. (author)

The role of grain boundary fission gases in high burn-up fuel under reactivity initiated accident conditions

International Nuclear Information System (INIS)

Lemoine, F.; Papin, J.; Frizonnet, J.M.; Cazalis, B.; Rigat, H.

2002-01-01

In the frame of reactivity-initiated accidents (RIA) studies, the CABRI REP-Na programme is currently performed, focused on high burn-up UO 2 and MOX fuel behaviour. From 1993 to 1998, seven tests were performed with UO 2 fuel and three with MOX fuel. In all these tests, particular attention has been devoted to the role of fission gases in transient fuel behaviour and in clad loading mechanisms. From the analysis of experimental results, some basic phenomena were identified and a better understanding of the transient fission gas behaviour was obtained in relation to the fuel and clad thermo-mechanical evolution in RIA, but also to the initial state of the fuel before the transient. A high burn-up effect linked to the increasing part of grain boundary gases is clearly evidenced in the final gas release, which would also significantly contribute to the clad loading mechanisms. (authors)

Advanced PWR Core Design with Siemens High-Plutonium-Content MOX Fuel Assemblies

International Nuclear Information System (INIS)

Dieter Porsch; Gerhard Schlosser; Hans-Dieter Berger

2000-01-01

The Siemens experience with plutonium recycling dates back to the late 1960s. Over the years, extensive research and development programs were performed for the qualification of mixed-oxide (MOX) technology and design methods. Today's typical reload enrichments for uranium and MOX fuel assemblies and modern core designs have become more demanding with respect to accuracy and reliability of design codes. This paper presents the status of plutonium recycling in operating high-burnup pressurized water reactor (PWR) cores. Based on actual examples, it describes the validation status of the design methods and stresses current and future needs for fuel assembly and core design including those related to the disposition of weapons-grade plutonium

Validation of the TUBRNP model with the radial distribution of plutonium in MOX fuel measured by SIMS and EPMA

Energy Technology Data Exchange (ETDEWEB)

O` Carroll, C; Laar, J Van De; Walker, C T [CEC Joint Research Centre, Karlsruhe (Germany)

1997-08-01

The new model TUBRNP (TRANSURANUS burnup) predicts the radial power density distribution as a function of burnup (and hence the radial burnup profile as a function of time) together with the radial profile of plutonium. Comparisons between measurements and the prediction of the TUBRNP model have been made for UO{sub 2} LWR fuels: they were found to be in excellent agreement and it is seen that TUBRNP is a marked improved on previous models. A powerful techniques for the characterization of irradiation fuel is Electron Probe Microanalysis (EPMA). Uranium, plutonium and fission product distributions can be analysed quantitatively. A complement, providing isotopic information with a lateral resolution comparable to EPMA, is secondary ion mass spectrometry (SIMS). Recently, the technique has been successfully applied for the measurement of the radial distribution of plutonium isotopes in irradiated nuclear fuel pins. The extension of the TUBRNP model to mixed oxide fuels seems to be the natural step to take. In MOX fuels the picture is greatly complicated by the presence of the (U, Pu)O{sub 2} agglomerates. The rim effect referred to above may be masked by the high concentrations of plutonium in the bulk of the fuel. A detailed investigation of a number of MOX fuel samples has been made using the TUBRNP model. Results are presented for a range of fuels with different enrichment and burnup. Through its participation in the PRIMO and DOMO programmes, PSI in conjunction with the Institute for Transuranium Elements had the opportunity to validate the new theoretical model TUBRNP. The authors with therefore to express their thanks to the organizers and to the numerous European and Japanese organizations which have supported these two international programmes on MOX fuel behavior. 7 refs, 9 figs, 3 tabs.

MOX fuel assembly and reactor core

International Nuclear Information System (INIS)

Shimada, Hidemitsu; Koyama, Jun-ichi; Aoyama, Motoo

1998-01-01

The MOX fuel assembly of the present invention is of a c-lattice type loaded to a BWR type reactor. 74 MOX fuel rods filled with mixed oxides of uranium and plutonium and two water rods disposed to a space equal to that for 7 MOX fuel rods are arranged in 9 x 9 matrix. MOX fuel rods having the lowest enrichment degree are disposed to four corners of the 9 x 9 matrix. The enrichment degree means a ratio of the weight of fission products based on the total weight of fuels. Two MOX fuel rods having the same enrichment degree are arranged in each direction so as to be continuous from the MOX fuel rods at four corners in the direction of the same row and different column and same column and the different row. In addition, among the outermost circumferential portion of the 9 x 9 matrix, MOX fuel rods having a lower enrichment degree next to the MOX fuel rods having the lowest enrichment degree are arranged, each by three to a portion where MOX fuel rods having the lowest enrichment degree are not disposed. (I.N.)

Present status and future developments of the implementation of burnup credit in spent fuel management systems in Germany

International Nuclear Information System (INIS)

Neuber, J.C.; Kuehl, H.

2001-01-01

This paper describes the experience gained in Germany in implementing burnup credit in wet storage and dry transport systems of spent PWR, BWR, and MOX fuel. It gives a survey of the levels of burnup credit presently used, the regulatory status and activities planned, the fuel depletion codes and criticality calculation codes employed, the verification methods used for validating these codes, the modeling assumptions made to ensure that the burnup credit criticality analysis is based on a fuel irradiation history which leads to bounding neutron multiplication factors, and the implementation of procedures used for fuel loading verification. (author)

Present status and future developments of the implementation of burnup credit in spent fuel management systems in Germany

Energy Technology Data Exchange (ETDEWEB)

Neuber, J C [Siemens Nuclear Power GmbH, Offenbach (Germany); Kuehl, H [Wissenschaftlich-Technische Ingenieurberatung WTI GmbH, Juelich (Germany)

2001-08-01

This paper describes the experience gained in Germany in implementing burnup credit in wet storage and dry transport systems of spent PWR, BWR, and MOX fuel. It gives a survey of the levels of burnup credit presently used, the regulatory status and activities planned, the fuel depletion codes and criticality calculation codes employed, the verification methods used for validating these codes, the modeling assumptions made to ensure that the burnup credit criticality analysis is based on a fuel irradiation history which leads to bounding neutron multiplication factors, and the implementation of procedures used for fuel loading verification. (author)

Analysis of Core Physics Experiments on Irradiated BWR MOX Fuel in REBUS Program

International Nuclear Information System (INIS)

Yamamoto, Toru; Ando, Yoshihira; Hayashi, Yamato

2008-01-01

As part of analyses of experimental data of a critical core containing a irradiated BWR MOX test bundle in the REBUS program, depletion calculations was performed for the BWR MOX fuel assemblies from that the MOX test rods were selected by using a general purpose neutronics code system SRAC. The core analyses were carried out using SRAC and a continuous energy Monte Carlo code MVP. The calculated k eff s were compared with those of the core containing a fresh MOX fuel bundle in the program. The SRAC-diffusion calculation underestimates k eff s of the both cores by 1.0 to 1.3 %dk and the k eff s of MVP are 1.001. The difference in k eff between the irradiated BWR MOX test bundle core and the fresh MOX one is 0.4 %dk in the SRAC-diffusion calculation and 0.0 %dk in the MVP calculation. The calculated fission rate distributions are in good agreement with the measurement in the SRAC-diffusion and MVP calculations. The calculated neutron flux distributions are also in good agreement with the measurement. The calculated burnup reactivity in the both calculations well reproduce the measurements. (authors)

Burnup simulations of an inert matrix fuel using a two region, multigroup reactor physics model

Energy Technology Data Exchange (ETDEWEB)

Schneider, E. [Dept. of Mechanical Engineering, Univ. of Texas at Austin, 1 Univ. Place C2200, Austin, TX 78712 (United States); Deinert, M.; Bingham Cady, K. [Dept. of Theoretical and Applied Mechanics, Cornell Univ., Ithaca, NY 14853 (United States)

2006-07-01

Determining the time dependent concentration of isotopes in a nuclear reactor core is of fundamental importance to analysis of nuclear fuel cycles and the impact of spent fuels on long term storage facilities. We present a fast, conceptually simple tool for performing burnup calculations applicable to obtaining isotopic balances as a function of fuel burnup. The code (VBUDS: visualization, burnup, depletion and spectra) uses a two region, multigroup collision probability model to determine the energy dependent neutron flux and tracks the buildup and burnout of 24 actinides, as well as fission products. The model has been tested against benchmarked results for LWRs burning UOX and MOX, as well as MONTEBURNS simulations of zirconium oxide based IMF, all with strong fidelity. As an illustrative example, VBUDS burnup calculation results for an IMF fuel are presented in this paper. (authors)

Numerical Tests for the Problem of U-Pu Fuel Burnup in Fuel Rod and Polycell Models Using the MCNP Code

Science.gov (United States)

Muratov, V. G.; Lopatkin, A. V.

An important aspect in the verification of the engineering techniques used in the safety analysis of MOX-fuelled reactors, is the preparation of test calculations to determine nuclide composition variations under irradiation and analysis of burnup problem errors resulting from various factors, such as, for instance, the effect of nuclear data uncertainties on nuclide concentration calculations. So far, no universally recognized tests have been devised. A calculation technique has been developed for solving the problem using the up-to-date calculation tools and the latest versions of nuclear libraries. Initially, in 1997, a code was drawn up in an effort under ISTC Project No. 116 to calculate the burnup in one VVER-1000 fuel rod, using the MCNP Code. Later on, the authors developed a computation technique which allows calculating fuel burnup in models of a fuel rod, or a fuel assembly, or the whole reactor. It became possible to apply it to fuel burnup in all types of nuclear reactors and subcritical blankets.

On the thermal evolution of Pu-rich agglomerates in MOX

International Nuclear Information System (INIS)

Verwerft, M.; Leenaers, A.; Lippens, M.; Mertens, L.

1999-01-01

From the experience accumulated so far on irradiated MOX fuel, its overall behaviour under irradiation is generally well predicted by existing fuel models. It appears however that additional data are still welcome to properly benchmark fission gas release models, mainly at elevated burnup. To this aim, an international research project, FIGARO, was initiated. Its goal was to provide thermal and fission gas release data og MOX at high burnup. Two MOX fuel rods irradiated to high burnup (50 GWd/tM peak pellet) but at lower power (less than 200 W/cm) were selected for segmentation and instrumentation with central thermocouple and pressure gauge. The instrumented segments were subjected to irradiations at variable linear power in the HALDEN MTR. Both temperature and internal pressure were online monitored during the ramp test. Afterwards, the rod segments were transported and extensively investigated. The paper focuses on the investigation of the evolution of the microstructure of Pu-rich agglomerates as a function of temperature

Transport of MOX fuel

International Nuclear Information System (INIS)

Porter, I.R.; Carr, M.

1997-01-01

The regulatory framework which governs the transport of MOX fuel is set out, including packages, transport modes and security requirements. Technical requirements for the packages are reviewed and BNFL's experience in plutonium and MOX fuel transport is described. The safety of such operations and the public perception of safety are described and the question of gaining public acceptance for MOX fuel transport is addressed. The paper concludes by emphasising the need for proactive programmes to improve the public acceptance of these operations. (Author)

A plan of reactor physics experiments for reduced-moderation water reactors with MOX fuel in TCA

International Nuclear Information System (INIS)

Shimada, Shoichiro; Akie, Hiroshi; Suzaki, Takenori; Okubo, Tutomu; Usui, Shuji; Shirakawa, Toshihisa; Iwamura, Takamiti; Kugo, Teruhiko; Ishikawa, Nobuyuki

2000-06-01

The Reduced-Moderation Water Reactor (RMWR) is one of the next generation water-cooled reactors which aim at effective utilization of uranium resource, high burn-up, long operation cycle, and plutonium multi-recycle. For verification of the feasibility, negative void reactivity coefficient and conversion ratio more than 1.0 must be confirmed. Critical Experiments performed so far in Eualope and Japan were reviewed, and no useful data are available for RMWR development. Critical experiments using TCA (Tank Type Critical Assembly) in JAERI are planned. MOX fuel rods should be prepared for the experiments and some modifications of the equipment are needed for use of MOX fuel rods. This report describes the preliminary plan of physics experiments. The number of MOX fuel rods used in the experiments are obtained by calculations and the modification of the equipment for the experiments are shown. (author)

Fission gas release of MOX with heterogeneous structure

International Nuclear Information System (INIS)

Nakae, N.; Akiyama, H.; Kamimura, K; Delville, R.; Jutier, F.; Verwerft, M.; Miura, H.; Baba, T.

2015-01-01

It is very useful for fuel integrity evaluation to accumulate knowledge base on fuel behavior of uranium and plutonium mixed oxide (MOX) fuel used in light water reactors (LWRs). Fission gas release is one of fuel behaviors which have an impact on fuel integrity evaluation. Fission gas release behavior of MOX fuels having heterogeneous structure is focused in this study. MOX fuel rods with a heterogeneous fuel microstructure were irradiated in Halden reactor (IFA-702) and the BR-3/BR-2 CALLISTO Loop (CHIPS program). The 85 Kr gamma spectrometry measurements were carried out in specific cycles in order to examine the concerned LHR (Linear Heat Rate) for fission gas release in the CHIPS program. The concerned LHR is defined in this paper to be the LHR at which a certain additional fission gas release thermally occurs. Post-irradiation examination was performed to understand the fission gas release behavior in connection with the pellet microstructure. The followings conclusions can be made from this study. First, the concerned LHR for fission gas release is estimated to be in the range of 20-23 kW/m with burnup over 37 GWd/tM. It is moreover guessed that the concerned LHR for fission gas release tends to decrease with increasing burnup. Secondly It is observed that FGR (fission gas release rate) is positively correlated with LHR when the LHR exceeds the concerned value. Thirdly, when burnup dependence of fission gas release is discussed, effective burnup should be taken into account. The effective burnup is defined as the burnup at which the LHR should be exceed the concerned value at the last time during all the irradiation period. And fourthly, it appears that FGR inside Pu spots is higher than outside and that retained (not released) fission gases mainly exist in the fission gas bubbles. Since fission gases in bubbles are considered to be easily released during fuel temperature increase, this information is very important to estimate fission gas release behavior

Verification of the depletion capabilities of the MCNPX code on a LWR MOX fuel assembly

International Nuclear Information System (INIS)

Cerba, S.; Hrncir, M.; Necas, V.

2012-01-01

The study deals with the verification of the depletion capabilities of the MCNPX code, which is a linked Monte-Carlo depletion code. For such a purpose the IV-B phase of the OECD NEA Burnup credit benchmark has been chosen. The mentioned benchmark is a code to code comparison of the multiplication coefficient k eff and the isotopic composition of a LWR MOX fuel assembly at three given burnup levels and after five years of cooling. The benchmark consists of 6 cases, 2 different Pu vectors and 3 geometry models, however in this study only the fuel assembly calculations with two Pu vectors were performed. The aim of this study was to compare the obtained result with data from the participants of the OECD NEA Burnup Credit project and confirm the burnup capability of the MCNPX code. (Authors)

Technology developments for Japanese BWR MOX fuel utilization

International Nuclear Information System (INIS)

Oguma, M.; Mochida, T.; Nomata, T.; Asahi, K.

1997-01-01

The Long-Term Program for Research, Development and Utilization of Nuclear Energy established by the Atomic Energy Commission of Japan asserts that Japan will promote systematic utilization of MOX fuel in LWRs. Based on this Japanese nuclear energy policy, we have been pushing development of MOX fuel technology aimed at future full scale utilization of this fuel in BWRs. In this paper, the main R and D topics are described from three subject areas, MOX core and fuel design, MOX fuel irradiation behaviour, and MOX fuel fabrication technology. For the first area, we explain the compatibility of MOX fuel with UO 2 core, the feasibility of the full MOX core, and the adaptability of MOX design methods based on a mock-up criticality experiment. In the second, we outline the Tsuruga MOX irradiation program and the DOMO program, and suggest that MOX fuel behaviour is comparable to ordinary BWR UO 2 fuel behaviour. In the third, we examine the development of a fully automated MOX bundle assembling apparatus and its features. (author). 14 refs, 11 figs, 3 tabs

Fuel component of electricity generation cost for the BN-800 reactor with MOX fuel and uranium oxide fuel with increasing of fuel burnup and removing of radial breeding blanket

International Nuclear Information System (INIS)

Raskach, A.

2001-01-01

Nowadays there are two completed design concepts of Nuclear Power Plants (NPPs) with the BN-800 type reactors developed with due regard for advanced safety requirements. One of them is the design of the fourth unit of the Beloyarsk Nuclear Power Plant; the other one is the design of three units of the South Ural Nuclear Power Plant. The both concepts are to use mixed oxide fuel (MOX fuel) based on civil plutonium. Studies on any project include economical analyses and cost of fuel is an essential parameter. In the course of the design works on the both projects such evaluations were done. For BN-800 on the Beloyarsk site nuclear fuel costs were taken from actual expenses of the BN-600 reactor and converted to rated thermal power and design capacity factor of the BN-800 and then increased by 20% in connection with turning to MOX fuel. Then this methodology was rewarding, but the ratio of uranium fuel and MOX fuel costs might change for the last years. For the project of three units of the South Ural Nuclear Power Plant nuclear fuel expenses were calculated from the data on a MOX fuel fabrication production facility (Complex-300). However, investigations performed recently shown that the methodology of economical assessments should be revised, as well as design and technology of MOX fuel fabrication at Complex-300 should be revised to meet all the existing safety requirements. Excepting there is a great bulk of civil plutonium to be reproduced, now we came up against the problem to utilize the exceeding ex-weapons plutonium that obviously can be used for MOX fuel fabrication as well. Construction of the MOX fuel fabrication facility - Complex-300 - was started in 1983. Its design output was planned to provide simultaneously 4 fast reactors of the BN-800 type with MOX fuel. By now about 50% of construction works (taking into account auxiliary buildings and arrangements) and 20% of installation works have been done at Complex-300. Along this, first works to construct

MOX fuel transport: the French experience

International Nuclear Information System (INIS)

Sanchis, H.; Verdier, A.; Sanchis, H.

1999-01-01

In the back-end of the fuel cycle, several leading countries have chosen the Reprocessing, Conditioning, Recycling (RCR) option. Plutonium recycling in the form of MOX fuel is a mature industry, with successful operational experience and large-scale fabrication plants an several European countries. The COGEMA Group has developed the industrialized products to master the RCR operation including transport COGEMA subsidiary, TRANSNUCLEAIRE has been operating MOX fuel transports on an industrial scale for more than 10 years. In 1998, around 200 transports of Plutonium materials have been organised by TRANSNUCLEAIRE. These transports have been carried out by road between various facilities in Europe: reprocessing plants, manufacturing plants and power plants. The materials transported are either: PuO 2 and MOX powder; BWR and PWR MOX fuel rods; BWR and PWR MOX fuel assemblies. Because MOX fuel transport is subject to specific safety, security and fuel integrity requirements, the MOX fuel transport system implemented by TRANSNUCLEAIRE is fully dedicated. Packaging have been developed, licensed and manufactured for each kind of MOX material in compliance with relevant regulations. A fleet of vehicles qualified according to existing physical protection regulations is operated by TRANSNUCLEAIRE. TRANSNUCLEAIRE has gained a broad experience in MOX transport in 10 years. Technical and operational know-how has been developed and improved for each step: vehicles and packaging design and qualification; vehicle and packaging maintenance; transport operations. Further developments are underway to increase the payload of the packaging and to improve the transport conditions, safety and security remaining of course top priority. (authors)

MOX use in PWRs. EDF operation experience

International Nuclear Information System (INIS)

Provost, Jean-Luc; Debes, Michel

2011-01-01

From the origin, EDF back-end fuel cycle strategy has focused on 'closing the fuel cycle', in other words integrating fuel reprocessing, with vitrification of high level waste concentrated within small volumes, and the recycling of valuable materials. The implementation of this policy was marked in 1987 by the first loading of sixteen MOX. By December 2010, 20 reactors have been loaded with 1750 tHM of MOX. EDF current strategy is to match the reprocessing program with MOX manufacturing capacity to limit the quantity of separated plutonium. This is routinely called the 'flow ad-equation' strategy. Currently, the MOX Parity core management achieves balance of MOX and UOX performance with a significant increase of the MOX discharge burn-up. Globally, the behavior under irradiation of MOX fuel assemblies has been satisfactory. So far, from the beginning of MOX use in EDF PWRs, only 6 MOX FAs with rod leakage have been identified, which gives a very satisfactory level of reliability. The industrial maturity of MOX fuel, with increased performances, allows the improvement of nuclear KWh competitiveness and of the plant operation performance, while maintaining in operation the same safety level, without significant impact on environment and radiological protection. (author)

MOX fuel fabrication at AECL

International Nuclear Information System (INIS)

Dimayuga, F.C.; Jeffs, A.T.

1995-01-01

Atomic Energy of Canada Limited's mixed-oxide (MOX) fuel fabrication activities are conducted in the Recycle Fuel Fabrication Laboratories (RFFL) at the Chalk River Laboratories. The RFFL facility is designed to produce experimental quantities of CANDU MOX fuel for reactor physics tests or demonstration irradiations. From 1979 to 1987, several MOX fuel fabrication campaigns were run in the RFFL, producing various quantities of fuel with different compositions. About 150 bundles, containing over three tonnes of MOX, were fabricated in the RFFL before operations in the facility were suspended. In late 1987, the RFFL was placed in a state of active standby, a condition where no fuel fabrication activities are conducted, but the monitoring and ventilation systems in the facility are maintained. Currently, a project to rehabilitate the RFFL and resume MOX fuel fabrication is nearing completion. This project is funded by the CANDU Owners' Group (COG). The initial fabrication campaign will consist of the production of thirty-eight 37-element (U,Pu)O 2 bundles containing 0.2 wt% Pu in Heavy Element (H.E.) destined for physics tests in the zero-power ZED-2 reactor. An overview of the Rehabilitation Project will be given. (author)

A PCI failure in an experimental MOX fuel rod and its sensitivity analysis

International Nuclear Information System (INIS)

Marino, A.C.

2000-01-01

Within our interest in studying MOX fuel performance, the irradiation of the first Argentine prototypes of PHWR MOX fuels began in 1986 with six rods fabricated at the α Facility (CNEA, Argentina). These experiences were made in the HFR-Petten reactor, Holland. The goal of this experience was to study the fuel behaviour with respect to PMCI-SCC. An experiment for extended burnup was performed with the last two MOX rods. During the experiment the final test ramp was interrupted due to a failure in the rod. The post-irradiation examinations indicated that PCI-SCC was a mechanism likely to produce the failure. At the Argentine Atomic Energy Commission (CNEA) the BACO code was developed for the simulation of a fuel rod thermo-mechanical behaviour under stationary and transient power situations. BACO includes a probability analysis within its structure. In BACO the criterion for safe operation of the fuel is based on the maximum hoop stress being below a critical value at the cladding inner surface; this is related to susceptibility to stress corrosion cracking (SCC). The parameters of the MOX irradiation, the preparation of the experiments and post-irradiation analysis were sustained by the BACO code predictions. We present in this paper an overview of the different experiences performed with the MOX fuel rods and the main findings of the post-irradiation examinations. A BACO code description, a wide set of examples which sustain the BACO code validation, and a special calculation for BU15 experiment attained using the BACO code, including a probabilistic analysis of the influence of rod parameters on performance, are included. (author)

Program on MOX fuel utilization in light water reactors

International Nuclear Information System (INIS)

Kenda, Hirofumi

2000-01-01

MOX fuel utilization program by the Japanese electric power companies was released in February, 1997. Principal philosophy for MOX fuel design is that MOX fuel shall be compatible with Uranium fuel and behavior of core loaded with MOX fuel shall be similar to that of conventional core. MOX fuel is designed so that geometry and nuclear capability of MOX fuel are equivalent to Uranium fuel. (author)

MOX fuel for Indian nuclear power programme

International Nuclear Information System (INIS)

Kamath, H.S.; Anantharaman, K.; Purushotham, D.S.C.

2000-01-01

A sound energy policy and a sound environmental policy calls for utilisation of plutonium (Pu) in nuclear power reactors. The paper discusses the use of Pu in the form of mixed oxide (MOX) fuel in two Indian boiling water reactors (BWRs) at Tarapur. An industrial scale MOX fuel fabrication plant is presently operational at Tarapur which is capable of manufacturing MOX fuels for BWRs and in future for PHWRs. The plant can also manufacture mixed oxide fuel for prototype fast breeder reactor (PFBR) and development work in this regard has already started. The paper describes the MOX fuel manufacturing technology and quality control techniques presently in use at the plant. The irradiation experience of the lead MOX assemblies in BWRs is also briefly discussed. The key areas of interest for future developments in MOX fuel fabrication technology and Pu utilisation are identified. (author)

BWRs with MOx fuel

International Nuclear Information System (INIS)

Demaziere, C.

1999-01-01

Calculations has been performed for loading BWRs with pure MOx or UOx/MOx fuel. It seems to be possible to load MOx bundles in BWRs, since most of the core characteristics are comparable with the ones of a full UOx core. Nevertheless two main problems arise: The shutdown margin at BOC is lower than 1%, this requires to have a new design for the control rods in order to increase their efficiency - but the problem can also be solved by modifying the Pu quality. The cores with MOx fuel are slightly less stable, unfortunately the simple model applied does not allow giving an absolute value for the decay ratio but only allows comparing the stability with the full UOx core

Recycling of MOX fuel for LWRs

International Nuclear Information System (INIS)

Joo, Hyung Kook; Oh, Soo Youl

1992-01-01

The status and issues related to the thermal recycling of reprocessed nuclear fuels have been reviewed. It is focused on the use of reprecessed plutonium in the form of mixed oxide (MOX) for a light water reactor and the review on reprocessing and fabrication processes is beyond the scope. In spite of the difference in the nuclear characteristics between plutonium and uranium isotopes, the neutronics behavior in a core with MOX fuels is similar to that with normal uranium fuels. However, since the neutron spectrum is hardened in a core with MOX, the Doppler, viod, and moderator temperature coefficients become more negative and the control rod and boron worths are slightly reduced. Therefore, the safety will be evaluated carefully in addition to the core neutronics analysis. The MOX fuel rod behavior related to the rod performance such as the pellet to clad interaction and fission gas release is also similar to that of uranium rods, and no specific problem arises. Substituting MOX fuels for a portion of uranium fuels, it is estimated that the savings be about 25% in uranium ore and 10% in uranium enrichment service requirements. The use of MOX fuel in LWRs has been commercialized in European countries including Germany, France, Belgium, etc., and a demonstration program has been pursued in Japan for the commercial utilization in the late 1990s. Such a worldwide trend indicates that the utilization of MOX fuel in LWRs is a proven technology and meets economics criteria. (Author)

Models for MOX fuel behaviour. A selective review

International Nuclear Information System (INIS)

Massih, Ali R.

2006-01-01

This report reviews the basic physical properties of light water reactor mixed-oxide (MOX) fuel comprising nuclear characteristics, thermal properties such as melting temperature, thermal conductivity, thermal expansion, and heat capacity, and compares these with properties of conventional UO 2 fuel. These properties are generally well understood for MOX fuel and are well described by appropriate models developed for engineering analysis. Moreover, certain modelling approaches of MOX fuel in-reactor behaviour, regarding densification, swelling, fission product gas release, helium release, fuel creep and grain growth, are evaluated and compared with the models for UO 2 . In MOX fuel the presence of plutonium rich agglomerates adds to the complexity of fuel behaviour on the micro scale. In addition, we survey the recent fuel performance experience and post irradiation examinations on several types of MOX fuel types. We discuss the data from these examinations, regarding densification, swelling, fission product gas release and the evolution of the microstructure during irradiation. The results of our review indicate that in general MOX fuel has a higher fission gas release and helium release than UO 2 fuel. Part of this increase is due to the higher operating temperatures of MOX fuel relative to UO 2 fuel due to the lower thermal conductivity of MOX material. But this effect by itself seems to be insufficient to make for the difference in the observed fission gas release of UO 2 vs. MOX fuel. Furthermore, the irradiation induced creep rate of MOX fuel is higher than that of UO 2 . This effect can reduce the pellet-clad interaction intensity in fuel rods. Finally, we suggest that certain physical based approaches discussed in the report are implemented in the fuel performance code to account for the behaviour of MOX fuel during irradiation

Models for MOX fuel behaviour. A selective review

Energy Technology Data Exchange (ETDEWEB)

Massih, Ali R. [Quantum Technologies AB, Uppsala Science Park (Sweden)

2006-12-15

This report reviews the basic physical properties of light water reactor mixed-oxide (MOX) fuel comprising nuclear characteristics, thermal properties such as melting temperature, thermal conductivity, thermal expansion, and heat capacity, and compares these with properties of conventional UO{sub 2} fuel. These properties are generally well understood for MOX fuel and are well described by appropriate models developed for engineering analysis. Moreover, certain modelling approaches of MOX fuel in-reactor behaviour, regarding densification, swelling, fission product gas release, helium release, fuel creep and grain growth, are evaluated and compared with the models for UO{sub 2}. In MOX fuel the presence of plutonium rich agglomerates adds to the complexity of fuel behaviour on the micro scale. In addition, we survey the recent fuel performance experience and post irradiation examinations on several types of MOX fuel types. We discuss the data from these examinations, regarding densification, swelling, fission product gas release and the evolution of the microstructure during irradiation. The results of our review indicate that in general MOX fuel has a higher fission gas release and helium release than UO{sub 2} fuel. Part of this increase is due to the higher operating temperatures of MOX fuel relative to UO{sub 2} fuel due to the lower thermal conductivity of MOX material. But this effect by itself seems to be insufficient to make for the difference in the observed fission gas release of UO{sub 2} vs. MOX fuel. Furthermore, the irradiation induced creep rate of MOX fuel is higher than that of UO{sub 2}. This effect can reduce the pellet-clad interaction intensity in fuel rods. Finally, we suggest that certain physical based approaches discussed in the report are implemented in the fuel performance code to account for the behaviour of MOX fuel during irradiation.

Advanced analysis technology for MOX fuel

International Nuclear Information System (INIS)

Hiyama, T.; Kamimura, K.

1997-01-01

PNC has developed MOX fuels for advanced thermal reactor (ATR) and fast breeder reactor (FBR). The MOX samples have been chemically analysed to characterize the MOX fuel for JOYO, MONJU, FUGEN and so on. The analysis of the MOX samples in glove box has required complicated and highly skilled operations. Therefore, for quality control analysis of the MOX fuel in a fabrication plant, simple, rapid and accurate analysis methods are necessary. To solve the above problems instrumental analysis and techniques were developed. This paper describes some of the recent developments in PNC. 2. Outline of recently developed analysis methods by PNC. 2.1 Determination of oxygen to metal atomic ratio (O/M) in MOX by non-dispersive infrared spectrophotometry after inert gas fusion. 7 refs, 9 figs, 4 tabs

Fuel cycle and waste management. 2. Design of a BWR Core with Over-moderated MOX Fuel Assemblies

International Nuclear Information System (INIS)

Francois, J.L.; Del Campo, C. Martin

2001-01-01

The use of uranium-plutonium mixed-oxide (MOX) fuel in light water reactors is a current practice in several countries. Generally one-third of the reactor core is loaded with MOX fuel assemblies, and the other two-thirds is loaded with uranium assemblies. Nevertheless, the plutonium utilization could be more effective if the full core could be loaded with MOX fuel. In this work, the design of a boiling water reactor (BWR) core fully loaded with over-moderated MOX fuel designs was investigated. In previous work, the design of over-moderated BWR MOX fuel assemblies based on a 10 x 10 lattice was presented; these designs improve the neutron spectrum and the plutonium consumption rate, compared with standard MOX assemblies. To increase the moderator-to-fuel ratio (MFR), two approaches were followed. In the first approach, 8 or 12 fuel rods were replaced by water rods in the 10x10 assembly, which increased the MFR from 1.9 to 2.2 and 2.4, respectively. These designs are called MOX-8WR and MOX-12WR, respectively, in this paper. In the second approach, an 11 x 11 lattice with 24 water rods (11 x 11-24WR) was designed, which is a design with a number of active fuel rods (88) very close to the standard MOX assembly (91). The fuel rod diameter is smaller to preserve the assembly dimensions, and in this last case, the MFR is 2.4. The calculations were performed with the CM-PRESTO three-dimensional steady-state simulator. The nuclear data banks were generated with the HELIOS system, and they were processed by TABGEN to produce tables of nuclear cross sections depending on burnup, void, and exposure weighted void (void history), which are used by CM-PRESTO. One base reload pattern was designed for a BWR/5 rated at 1931 MW(thermal), to be used with the different over-moderated assembly designs. The reload pattern has 112 fresh fuel assemblies (FFAs) out of a total of 444 fuel assemblies and was simulated during 20 cycles with the Haling strategy, until an equilibrium cycle of

Instant release of fission products in leaching experiments with high burn-up nuclear fuels in the framework of the Euratom project FIRST- Nuclides

Energy Technology Data Exchange (ETDEWEB)

Lemmens, K., E-mail: klemmens@sckcen.be [Waste and Disposal Expert Group, Belgian Nuclear Research Centre (SCK-CEN), Boeretang 200, 2400 Mol (Belgium); González-Robles, E.; Kienzler, B. [Karlsruhe Institute of Technology Institute for Nuclear Waste Disposal (KIT-INE), PO Box 3640, D-76021 Karlsruhe (Germany); Curti, E. [Laboratory for Waste Management, Nuclear Energy and Safety Dept., Paul Scherrer Institute, 5232 Villigen PSI (Switzerland); Serrano-Purroy, D. [European Commission, DG Joint Research Centre - JRC, Directorate G - Nuclear Safety & Security, Department G.III, PO Box 2340, D-76125 Karlsruhe (Germany); Sureda, R.; Martínez-Torrents, A. [CTM Centre Tecnològic, Plaça de la Ciència 2, 08243 Manresa (Spain); Roth, O. [Studsvik, Nuclear AB, 611 82 Nyköping (Sweden); Slonszki, E. [Magyar Tudományos Akadémia Energiatudományi Kutatóközpont (MTA EK), PO Box 49, H-1525 Budapest (Hungary); Mennecart, T. [Waste and Disposal Expert Group, Belgian Nuclear Research Centre (SCK-CEN), Boeretang 200, 2400 Mol (Belgium); Günther-Leopold, I. [Laboratory for Waste Management, Nuclear Energy and Safety Dept., Paul Scherrer Institute, 5232 Villigen PSI (Switzerland); Hózer, Z. [Magyar Tudományos Akadémia Energiatudományi Kutatóközpont (MTA EK), PO Box 49, H-1525 Budapest (Hungary)

2017-02-15

The instant release of fission products from high burn-up UO{sub 2} fuels and one MOX fuel was investigated by means of leach tests. The samples covered PWR and BWR fuels at average rod burn-up in the range of 45–63 GWd/t{sub HM} and included clad fuel segments, fuel segments with opened cladding, fuel fragments and fuel powder. The tests were performed with sodium chloride – bicarbonate solutions under oxidizing conditions and, for one test, in reducing Ar/H{sub 2} atmosphere. The iodine and cesium release could be partially explained by the differences in sample preparation, leading to different sizes and properties of the exposed surface areas. Iodine and cesium releases tend to correlate with FGR and linear power rating, but the scatter of the data is significant. Although the gap between the fuel and the cladding was closed in some high burn-up samples, fissures still provide possible preferential transport pathways. - Highlights: • Leach tests were performed to study the instant release of fission products from high burn-up UO{sub 2} fuels and one MOX fuel. • In these tests, the fission gas release given by the operator was a pessimistic estimator of the iodine and cesium release. • Iodine and cesium release is proportional to linear power rating beyond 200 W cm{sup −1}. • Closure of the fuel-cladding gap at high burn-up slows down the release. • The release rate decreases following an exponential equation.

Development of vibropac MOX fuel pins serviceable up TP superhigh burnups

International Nuclear Information System (INIS)

Mayorshin, A.A.; Gadzhiev, G.I.; Kisly, V.A.; Skiba, O.V.; Tzykanov, V.A.

1998-01-01

The main results on investigations of fast reactor fuel pins with (UPu)O 2 vibropac fuel to substantiate their serviceability up to the super-high burnups are presented. The BOR-60 reactor fuel pins radiation behaviour in stationary, transient and designed emergency conditions has been determined from the fuel pins dimensional stability analysis having regard to the results of investigation fuel and cladding swelling as well as estimations of fuel and cladding thermal-mechanical and physico-chemical interactions. It is shown that the change of the outer diameter is minimum in fuel pins with VMOX fuel with a getter-metallic uranium powder and ferrito-martensite steel cladding, and the corrosion damage of the cladding inner surface is absent up to 26% h.a. The experiments with over-heating of the irradiated fuel pins cladding up to 850 deg. C did not lead to any changes in pins integrity. The availability of the periphery area of the vibropac fuel cure initial structure provides the minimum level of the thermal-mechanical stress at transient conditions of reactor operation. (author)

MX 8: the next generation high capacity system for the transport of fresh MOX fuel

International Nuclear Information System (INIS)

Potelle, F.; Issard, H.

1998-01-01

The choice of reprocessing policy was made a long time ago in France, leading to the development of an advanced Pu recycling industry. In 1987, Saint Laurent was the first French reactor to be loaded with fresh MOX fuel. Transnucleaire, then in charge of transport packaging development, created the FS 69 concept, derived from the classical RCC concept for the transport of UO 2 fresh fuel. On the other hand, Cogema, as the main actor in the field of fuel cycle and thus in transport matters, developed the associated security truck and security caisson in order to provide the transport system with the acceptable Physical Protection devices required by French Authorities. As a whole, the security truck and the FS 69 have now been used for more than ten years with a remarkable level of efficiency and safety. Indeed, more than 600 fresh MOX fuel elements have been delivered, without any incident, both regarding safety or fuel integrity requirements. But, as a matter of fact, the replacement of FS 69 transport system is now scheduled for several reasons. First of all, the burnups achieved with UO 2 fuel progressed together with its enrichment within the last ten years, and the MOX 'equivalence' also implies that its Pu content be increased to enhance its reactor performances: from 5.25 % of Pu content today, the MOX fuel will reach 7% tomorrow, and almost 10% the day after tomorrow. Lastly, the reprocessing/recycling policy has been confirmed and amplified, leading to an increasing number of 'moxified' reactors. As a consequence, the French utility (EDF), the fuel designer (Fragema, the joint venture between Framatome and Cogema), the fuel manufacturer (Cogema), and the transporter (Transnucleaire) joined in a specific working group devoted to the development of the MX 8, the next generation high capacity system for the land transport of MOX fuel. (authors)

A technique of melting temperature measurement and its application for irradiated high-burnup MOX fuels

International Nuclear Information System (INIS)

Namekawa, Takashi; Hirosawa, Takashi

1999-01-01

A melting temperature measurement technique for irradiated oxide fuels is described. In this technique, the melting temperature was determined from a thermal arrest on a heating curve of the specimen which was enclosed in a tungsten capsule to maintain constant chemical composition of the specimen during measurement. The measurement apparatus was installed in an alpha-tight steel box within a gamma-shielding cell and operated by remote handling. The temperature of the specimen was measured with a two-color pyrometer sighted on a black-body well at the bottom of the tungsten capsule. The diameter of the black-body well was optimized so that the uncertainties of measurement were reduced. To calibrate the measured temperature, two reference melting temperature materials, tantalum and molybdenum, were encapsulated and run before and after every oxide fuel test. The melting temperature data on fast reactor mixed oxide fuels irradiated up to 124 GWd/t were obtained. In addition, simulated high-burnup mixed oxide fuel up to 250 GWd/t by adding non-radioactive soluble fission products was examined. These data shows that the melting temperature decrease with increasing burnup and saturated at high burnup region. (author)

Public acceptance of MOX - fuel

International Nuclear Information System (INIS)

Huettmann, A.; Reddehase, C.G.

1995-01-01

In the Federal Republic of Germany 'Plutonium-Business' got fresh nutrient because of the carried out licensing of the use of Mixed Oxide (MOX)-fuel LWR and in connection with the negative attitude of the Hessian authorities, who are responsible for the licensing procedures of the production of MOX-fuel in the Siemens-factories at Hanau. The opponents of the peaceful use of nuclear energy try with the emotive expression 'Plutonium' (Pu) a frontal attack against the use of nuclear energy in Germany. They justify their actions with so-called safety deficits of the plants and increased danger of cancer in case of using MOX-fuel. (orig./HP)

Transport of MOX fuel from Europe to Japan

International Nuclear Information System (INIS)

2002-01-01

The MOX fuel transports from Europe to Japan represent a main part in the implementing of the Japan nuclear program. They complement the 160 transports of spent fuels realized from Japan to Europe and the vitrified residues return from France to Japan. In this framework the document presents the MOX fuel, the use of the MOX fuel in reactor, the proliferation risks, the MOX fuel transport to Japan, the public health, the transport regulations, the safety and the civil liability. (A.L.B.)

Top-MOX fuel solution: strategies, challenges, opportunities

International Nuclear Information System (INIS)

Breitenstein, P.; Vo Van, V.

2014-01-01

TOP-MOX is a nuclear fuel solution and product developed by AREVA and successfully implemented in Europe. It allows utilities burning plutonium (instead of enriched uranium) even when this plutonium is not stemming from own reprocessed used fuel - that is third party plutonium. The important challenges for utilities along with TOP-MOX implementation are legal/patrimonial Pu-ownership issues and general economical aspects. Available sponsorship of such plutonium permits UO2 competitive market prices. For new MOX customers licensing and technical aspects come along. Further AREVA proposes a flexible solution which is called 'TOP-MOX pre-cycling'. This involves making available third party plutonium for fuel fabrication and reactor use pending the utilities' final strategic fuel cycle decision. The paper gives insight into and analyses the impacts of allowing customers the implementation of a TOP-MOX program with focus on Pu-ownership, economics, technical and legal aspects as well as the impact on used MOX management and final waste management. (authors)

Advances in fuel pellet technology for improved performance at high burnup. Proceedings of a Technical Committee meeting

International Nuclear Information System (INIS)

1998-08-01

The IAEA has recently completed two co-ordinated Research Programmes (CRPs) on The Development of Computer Models for Fuel Element Behaviour in Water Reactors, and on Fuel Modelling at Extended Burnup. Through these CRPs it became evident that there was a need to obtain data on fuel behaviour at high burnup. Data related o thermal behaviour, fission gas release and pellet to clad mechanical interaction were obtained and presented at the Technical Committee Meeting on Advances in Fuel Pellet Technology for Improved Performance at High Burnup which was recommended by the International Working Group on Fuel Performance and Technology (IWGFPT). The 34 papers from 10 countries are published in this proceedings and presented by a separate abstract. The papers were grouped in 6 sessions. First two sessions covered the fabrication of both UO 2 fuel and additives and MOX fuel. Sessions 3 and 4 covered the thermal behaviour of both types of fuel. The remaining two sessions dealt with fission gas release and the mechanical aspects of pellet to clad interaction

MOX in reactors: present and future

International Nuclear Information System (INIS)

Arslan, Marc; Gros, Jean Pierre; Niquille, Aurelie; Marincic, Alexis

2010-01-01

In Europe, MOX fuel has been supplied by AREVA for more than 30 years, to 36 reactors: 21 in France, 10 in Germany, 3 in Switzerland, 2 in Belgium. For the present and future, recycling is compulsory in the frame of sustainable development of nuclear energy. By 2030 the overall volume of used fuel will reach about 400 000 t worldwide. Their plutonium and uranium content represents a huge resource of energy to recycle. That is the reason why, the European Utilities issued an EUR (European Utilities Requirement) demanding new builds reactors to be able of using MOX Fuel Assemblies in up to 50 % of the core. AREVA GEN3+ reactors, like EPR TM or ATMEA TM designed with MHI partnership, are designed to answer any utility need of MOX recycling. The example of the EPR TM reactor operated with 100 % MOX core optimized for MOX recycling will be presented. A standard EPR TM can be operated with 100 % MOX core using an advanced homogeneous MOX (single Pu content) with highly improved performances (burn-up and Cycle length). The adaptations needed and the main operating and safety reactor features will be presented. AREVA offers the utilities throughout the world, fuel supply (UO 2 , ERU, MOX), and reactors designed with all the needed capability for recycling. For each country and each utility, an adapted global solution, competitive and non proliferant can be proposed. (authors)

MOX fuel fabrication, in reactor performance and improvement

International Nuclear Information System (INIS)

Vliet, J. van; Deramaix, P.; Nigon, J.L.; Fournier, W.

1998-01-01

In Europe, MOX fuel for light water reactors (LWRs) has first been manufactured in Belgium and Germany. Belgonucleaire (BN) loaded the first MOX assembly in the BR3 Pressurised Water Reactor (PWR) in 1963. In June 1998, more than 750 tHM LWR MOX fuel assemblies were manufactured on a industrial scale in Europe without any particular difficulty relating to fuel fabrication, reactor operation or fuel behaviour. So, today plutonium recycling through MOX fuel is a mature industry, with successful operational experience and large-scale fabrication plants. In this field, COGEMA and BELGONUCLEAIRE are the main actors by operating simultaneously three complete multidesign fuel production plants: MELOX plant (in Marcoule), CADARACHE plant and P0 plant (in Dessel, Belgium). Present MOX production capacity available to COGEMA and BN fits 175 tHM per year and is to be extended to reach about 325 tHM in the year 2000. This will represent 75% of the total MOX fabrication capacity in Europe. The industrial mastery and the high production level in MOX fabrication assured by high technology processes confer to these companies a large expertise for Pu recycling. This allows COGEMA and BN to be major actors in Pu-based fuels in the coming second nuclear era with advanced fuel cycles. (author)

Preliminary nuclear design for test MOX Fuel rods

Energy Technology Data Exchange (ETDEWEB)

Joo, Hyung Kook; Kim, Taek Kyum; Jeong, Hyung Guk; Noh, Jae Man; Cho, Jin Young; Kim, Young Il; Kim, Young Jin; Sohn, Dong Seong

1997-10-01

As a part of activity for future fuel development project, test MOX fuel rods are going to be loaded and irradiated in Halden reactor core as a KAERI`s joint international program with Paul Scherrer Institute (PSI). PSI will fabricate test MOX rods with attrition mill device which was developed by KAERI. The test fuel assembly rig contains three MOX rods and three inert matrix rods. One of three MOX rods will be fabricated by BNFL, the other two MOX fuel rods will be manufacturing jointly by KAERI and PSI. Three inert matrix fuel rods will be fabricated with Zr-Y-Er-Pu oxide. Neutronic evaluation was preliminarily performed for test fuel assembly suggested by PSI. The power distribution of test fuel rod in test fuel assembly was analyzed for various fuel rods position in assembly and the depletion characteristic curve for test fuel was also determined. The fuel rods position in test fuel assembly does not effect the rod power distribution, and the proposal for test fuel rods suggested by PSI is proved to be feasible. (author). 2 refs., 13 tabs., 16 figs.

MOX fuel fabrication: Technical and industrial developments

International Nuclear Information System (INIS)

Lebastard, G.; Bairiot, H.

1990-01-01

The plutonium available in the near future is generally estimated rather precisely on the basis of the reprocessing contracts and the performance of the reprocessing plants. A few years ago, decision makers were convinced that a significant share of this fissile material would be used as the feed material for fast breeder reactors (FBRs) or other advanced reactors. The facts today are that large reprocessing plants are coming into commercial operations: UP3 and soon UP2-800 and THORP, but that FBR deployment is delayed worldwide. As a consequence, large quantities of plutonium will be recycled in light water reactors as mixed oxide (MOX) fuels. MOX fuel technology has been properly demonstrated in the past 25 years. All specific problems have been addressed, efficient fabrication processes and engineering background have been implemented to a level of maturity which makes MOX fuel behaving as well as Uranium fuel. The paper concentrates on todays MOX fabrication expertise and presents the technical and industrial developments prepared by the MOX fuel fabrication industry for this last decade of the century

Progress in researches on MOX fuel pellet producing technology in China

International Nuclear Information System (INIS)

Hu Xiaodan

2010-01-01

Being the key section of nuclear-fuel cycle, the producing technology of MOX(UO 2 -PuO 2 ) fuel had driven to maturity in France, England, Russia, Belgium, etc. MOX fuel had been applied in FBR and LWR successfully in those countries. With the rapidly developing of nuclear-generated power, the MOX fuel for FBR and LWR was active demanded in China. However, the producing technology of MOX fuel developed slowly. During the period of 'the seventh five year's project', MOX fuel pellet was produced by mechanically mixed method and oxalate deposited method, respectively. Parts of cool performance of MOX fuel pellet produced by oxalate deposited method reached the qualification of fuel for FBR. During the period of 'the ninth five year's project' and 'the tenth five year's project', the technical route of producing MOX fuel was determined, and the test line of producing MOX fuel was built preliminarily. In the same time, the producing technology and analyzing technology of MOX fuel pellet by mechanically mixed was studied roundly, and the representative analogue pellet(UO 2 -CeO 2 ) was produced. That settled the supporting technology for the commercial process and research of MOX fuel rod and MOX fuel module. (authors)

Transport of MOX fuel from Europe to Japan; Transport de combustible mox d' Europe vers le Japon

Energy Technology Data Exchange (ETDEWEB)

NONE

2002-07-01

The MOX fuel transports from Europe to Japan represent a main part in the implementing of the Japan nuclear program. They complement the 160 transports of spent fuels realized from Japan to Europe and the vitrified residues return from France to Japan. In this framework the document presents the MOX fuel, the use of the MOX fuel in reactor, the proliferation risks, the MOX fuel transport to Japan, the public health, the transport regulations, the safety and the civil liability. (A.L.B.)

Features of fuel performance at high fuel burnups

International Nuclear Information System (INIS)

Proselkov, V.N.; Scheglov, A.S.; Smirnov, A.V.; Smirnov, V.P.

2001-01-01

Some features of fuel behavior at high fuel burnups, in particular, initiation and development of rim-layer, increase in the rate of fission gas release from the fuel and increase in the inner gas pressure in the fuel rod are briefly described. Basing on the analysis of the data of post-irradiation examinations of fuel rods of WWER-440 working FA and CR fuel followers, that have been operated for five fuel cycles and got the average fuel burnup or varies as 50MW-day/kgU, a conclusion is made that the WWER-440 fuel burnup can be increased at least to average burnups of 55-58 MW-day/kgU per fuel assembly (Authors)

Performance of MOX fuel: An overview of the experimental programme of the OECD Halden Reactor Project and review of selected results

International Nuclear Information System (INIS)

Wiesenack, W.; McGrath, M.

2000-01-01

The OECD Halden Reactor Project has defined an extensive experimental programme related to MOX fuels which is being executed with the objective to provide a performance data base similar to that available for UO 2 . In addition to utilising fresh MOX fuel and re-instrumented segments from LWR irradiations to high burnup, the concept of inert matrix fuel is being addressed. The irradiation in the Halden reactor is performed in rigs allowing steady state, power ramping and cyclic operation. In-pile data are obtained from instrumentation such as fuel centreline thermocouples, pressure transducers, fuel and cladding elongation detectors, and movable gauges for measuring the diametral deformation. Various phenomena can be assessed in this way, e.g. thermal performance, swelling and densification, PCMI and fission gas release. The paper describes the objectives of various experiments and provides examples of temperature, pressure and cladding elongation measurements performed on MOX fuel. Salient results are related to the threshold for the onset of significant fission gas release and the relaxation behaviour in a power ramp-PCMI situation. (author)

Power ramp tests of BWR-MOX fuels

International Nuclear Information System (INIS)

Asahi, K.; Oguma, M.; Higuchi, S.; Kamimua, K.; Shirai, Y.; Bodart, S.; Mertens, L.

1996-01-01

Power ramp test of BWR-MOX and UO 2 fuel rods base irradiated up to about 60 GWd/t in Dodewaard reactor have been conducted in BR2 reactor in the framework of the international DOMO programme. The MOX pellets were provided by BN (MIMAS process) and PNC (MH method). The MOX fuel rods with Zr-liner and non-liner cladding and the UO 2 fuel rods with Zr-liner cladding remained intact during the stepwise power ramp tests to about 600 W/cm, even at about 60 GWd/t

A PWR Thorium Pin Cell Burnup Benchmark

Energy Technology Data Exchange (ETDEWEB)

Weaver, Kevan Dean; Zhao, X.; Pilat, E. E; Hejzlar, P.

2000-05-01

As part of work to evaluate the potential benefits of using thorium in LWR fuel, a thorium fueled benchmark comparison was made in this study between state-of-the-art codes, MOCUP (MCNP4B + ORIGEN2), and CASMO-4 for burnup calculations. The MOCUP runs were done individually at MIT and INEEL, using the same model but with some differences in techniques and cross section libraries. Eigenvalue and isotope concentrations were compared on a PWR pin cell model up to high burnup. The eigenvalue comparison as a function of burnup is good: the maximum difference is within 2% and the average absolute difference less than 1%. The isotope concentration comparisons are better than a set of MOX fuel benchmarks and comparable to a set of uranium fuel benchmarks reported in the literature. The actinide and fission product data sources used in the MOCUP burnup calculations for a typical thorium fuel are documented. Reasons for code vs code differences are analyzed and discussed.

Foundations for the definition of MOX fuel quality requirements

International Nuclear Information System (INIS)

Bairiot, H.; Deramaix, P.; Vanderborck, Y.

1991-01-01

The quality of uranium-plutonium mixed oxide (MOX) fuel, as of any nuclear fuel, depends on the design optimization and on the fabrication process stability. The design optimization is essentially based on feed-back from irradiation experience through engineering assessment of the results; the stability of the process is necessary to justify minimal uncertainty margins in the fuel design. Since MOX fuel is quite similar to UO 2 fuel, the lessons learned from UO 2 fuels can complement the MOX experimental data base. MOX is however different from UO 2 fuel in some respects, among others: the industrial fabrication scale is a factor 10 lower than for UO 2 fuel, the fuel enrichment process takes place in the manufacturing plant, the radioactivity of Pu imposes handling constraints, Pu ages quite rapidly, altering its isotopic composition during storage, the incorporation of Pu alters the material physics and neutronic characteristics of the fuel. In this perspective, the paper outlines some quality attributes for which MOX fuel may or even must depart form UO 2 fuel. (orig.)

Transport of MOX fuel from Europe to Japan; Transport de combustible mox d' Europe vers le Japon

Energy Technology Data Exchange (ETDEWEB)

NONE

2002-07-01

The MOX fuel transports from Europe to Japan represent a main part in the implementing of the Japan nuclear program. They complement the 160 transports of spent fuels realized from Japan to Europe and the vitrified residues return from France to Japan. In this framework the document presents the MOX fuel, the use of the MOX fuel in reactor, the proliferation risks, the MOX fuel transport to Japan, the public health, the transport regulations, the safety and the civil liability. (A.L.B.)

Isotopic modelling using the ENIGMA-B fuel performance code

International Nuclear Information System (INIS)

Rossiter, G.D.; Cook, P.M.A.; Weston, R.

2001-01-01

A number of experimental programmes by BNFL and other MOX fabricators have now shown that the in-pile performance of MOX fuel is generally similar to that of conventional UO 2 fuel. Models based on UO 2 fuel experience form a good basis for a description of MOX fuel behaviour. However, an area where the performance of MOX fuel is sufficiently different from that of UO 2 to warrant model changes is in the radial power and burnup profile. The differences in radial power and burnup profile arise from the presence of significant concentrations of plutonium in MOX fuel, at beginning of life, and their subsequent evolution with burnup. Amongst other effects, plutonium has a greater neutron absorption cross-section than uranium. This paper focuses on the development of a new model for the radial power and burnup profile within a UO 2 or MOX fuel rod, in which the underlying fissile isotope concentration distributions are tracked during irradiation. The new model has been incorporated into the ENIGMA-B fuel performance code and has been extended to track the isotopic concentrations of the fission gases, xenon and krypton. The calculated distributions have been validated against results from rod puncture measurements and electron probe micro-analysis (EPMA) linescans, performed during the M501 post irradiation examination (PIE) programme. The predicted gas inventory of the fuel/clad gap is compared with the isotopic composition measured during rod puncture and the measured radial distributions of burnup (from neodymium measurements) and plutonium in the fuel are compared with the calculated distributions. It is shown that there is good agreement between the code predictions and the measurements. (author)

Issues in the use of Weapons-Grade MOX Fuel in VVER-1000 Nuclear Reactors: Comparison of UO2 and MOX Fuels

Energy Technology Data Exchange (ETDEWEB)

Carbajo, J.J.

2005-05-27

The purpose of this report is to quantify the differences between mixed oxide (MOX) and low-enriched uranium (LEU) fuels and to assess in reasonable detail the potential impacts of MOX fuel use in VVER-1000 nuclear power plants in Russia. This report is a generic tool to assist in the identification of plant modifications that may be required to accommodate receiving, storing, handling, irradiating, and disposing of MOX fuel in VVER-1000 reactors. The report is based on information from work performed by Russian and U.S. institutions. The report quantifies each issue, and the differences between LEU and MOX fuels are described as accurately as possible, given the current sources of data.

Pyro-electrochemical reprocessing of irradiated MOX fast reactor fuel, testing of the reprocessing process with direct MOX fuel production

Energy Technology Data Exchange (ETDEWEB)

Kormilitzyn, M.V.; Vavilov, S.K.; Bychkov, A.V.; Skiba, O.V.; Chistyakov, V.M.; Tselichshev, I.V

2000-07-01

One of the advanced technologies for fast reactor fuel recycle is pyro-electrochemical molten salt technology. In 1998 we began to study the next phase of the irradiated oxide fuel reprocessing new process MOX {yields} MOX. This process involves the following steps: - Dissolution of irradiated fuel in molten alkaline metal chlorides, - Purification of melt from fission products that are co-deposited with uranium and plutonium oxides, - Electrochemical co-deposition of uranium and plutonium oxides under the controlled cathode potential, - Production of granulated MOX (crushing,salt separation and sizing), and - Purification of melt from fission products by phosphate precipitation. In 1998 a series of experiments were prepared and carried out in order to validate this process. It was shown that the proposed reprocessing flowsheet of irradiated MOX fuel verified the feasibility of its decontamination from most of its fission products (rare earths, cesium) and minor-actinides (americium, curium)

Pyro-electrochemical reprocessing of irradiated MOX fast reactor fuel, testing of the reprocessing process with direct MOX fuel production

International Nuclear Information System (INIS)

Kormilitzyn, M.V.; Vavilov, S.K.; Bychkov, A.V.; Skiba, O.V.; Chistyakov, V.M.; Tselichshev, I.V.

2000-01-01

One of the advanced technologies for fast reactor fuel recycle is pyro-electrochemical molten salt technology. In 1998 we began to study the next phase of the irradiated oxide fuel reprocessing new process MOX → MOX. This process involves the following steps: - Dissolution of irradiated fuel in molten alkaline metal chlorides, - Purification of melt from fission products that are co-deposited with uranium and plutonium oxides, - Electrochemical co-deposition of uranium and plutonium oxides under the controlled cathode potential, - Production of granulated MOX (crushing,salt separation and sizing), and - Purification of melt from fission products by phosphate precipitation. In 1998 a series of experiments were prepared and carried out in order to validate this process. It was shown that the proposed reprocessing flowsheet of irradiated MOX fuel verified the feasibility of its decontamination from most of its fission products (rare earths, cesium) and minor-actinides (americium, curium)

Development of MOX facilities and the impact on the nuclear fuel markets

International Nuclear Information System (INIS)

Patterson, J.

1990-01-01

Mixed-oxide (MOX) fuel is nearing maturity as a fuel supply option. This paper briefly reviews the history and current status of the MOX fuel market, including the projected increase in demand for MOX fuel as more plutonium becomes available from the operation of commercial irradiated fuel reprocessing plants in Europe. The uncertainties of such projected demand are discussed, together with the anticipated requirements from the next generation of MOX fabrication plants. The impact of the growing demand for MOX fuel is assessed in the traditional sectors of the uranium fuel cycle. Finally, the author turns to a generalized treatment of the economic aspects of MOX fuel utilization, showing the financially attractive regimes of MOX use which will benefit nuclear power utilities and continue to ensure that MOX fuel can consolidate its position as a mature fuel supply option in those countries that have opted to recycle their spent fuel

Study on high performance MOX fuel and core design in full MOX ABWR(1) by GNF-J

International Nuclear Information System (INIS)

Izutsu, Sadayuki; Goto, Daisuke; Saeki, Jun; Kokubun, Takehiro; Yokoya, Jun

2003-01-01

The concepts of high-performance MOX fuel using 10x10 lattices suitable for full-MOX ABWR are shown in this paper, in which average discharge exposure is extended up to 45 GWd/t with heavy-metal inventory increased over current MOX, reducing the number of refueling bundles, resulting in fuel cycle cost reduction and core performance satisfaction. Also, the increase of Pu inventory is taken into account from the viewpoint to extend the flexibility of MOX fuel utilization. (author)

Overview of MOX fuel fabrication achievements

International Nuclear Information System (INIS)

Bairiot, H.; Vliet, J. van; Chiarelli, G.; Edwards, J.; Nagai, S.H.; Reshetnikov, F.

2000-01-01

Such overview having been adequately covered in an OECD/NEA publication providing the situation as of end 1994, this paper is mainly devoted to an update as of end 1998. The Belgian plant, Belgonucleaire/Dessel, is now dedicated exclusively to the fabrication of MOX fuel and has operated consistently around its nameplate capacity (35tHM/a) through the 1990s involving a large variety of PWR and BWR fuels. The two French plants have also achieved routine operation during the 1990s. CFCa, historically the largest FBR MOX fuel manufacturer, is utilizing the genuine COCA process for that type of fuel and the MIMAS process for LWR fuel: a nominal capacity (40 tHM/a) has been gradually approached. MELOX has operated at 100 tHM/a, as defined in the operating licence granted originally. The British plant, MDF/Sellafield with 8tHM/a nameplate capacity is devoted to fuel and has manufactured several small fabrication campaigns. In Japan, JNC operates three facilities located at Tokai: PFDF, devoted to basic research and fabrication of test fuels, PFFF/ATR line, for the fabrication of Fugen fuel and of corresponding fuel for the critical facility DCA, and PFPF for the fabrication of FBR fuel. In Russia, fabrication techniques have been developed to fuel four BN-800 FBRs contemplated to be constructed and be fuelled with the civilian Pu stockpile. Two demonstration facilities Paket (Mayak) and RIAR (Dimitrovgrad) fabricated respectively pellet and vipac type FBR MOX fuel for BR-5, BOR-60, BN-350 and BN-600. The paper includes a brief description of each of the fabrication routes mentioned, as well as the production of respectively LWR and FBR MOX fuel in each fabrication facility, since the start-up of the plant, since 1 January 1993 and since 1 January 1998 up to 31 December 1998. (author)

MOX fuel fabrication and utilisation in LWRs worldwide

International Nuclear Information System (INIS)

Provost, J.-L.; Schrader, M.; Nomura, S.

2000-01-01

Early in the development of the nuclear programme, a large part of the countries using nuclear energy has studied the reprocessing and recycling option in order to develop a safe conditioning of fission products and to recycle fissile materials in reactors. In the sixties, the feasibility of recycling plutonium in LWRs has been successfully demonstrated by several experimentations of MOX rod irradiations in different countries. Based on the background of the MOX behaviour collected during the seventies and on the results of the important MOX experimentation program implemented during this period, a large part of the European utilities decided at the beginning of the eighties to use MOX fuel in LWRs on an industrial scale. The main goals of the utilities were to use as a fuel an available fissile material and to control the stockpile of separated plutonium. Today, the understanding of the behaviour of plutonium fuel has grown significantly since the launch of the first R and D programmes on LWR and FR MOX fuels. Plutonium oxide physical and neutron behaviour is well known, its modelling is now available as well as experimentally validated. Up to now, more than 750 tHM MOX fuel (more than 2000 FAs) have been loaded in 29 PWRs and in 2 BWRs in Europe, corresponding to the recycling of about 35 t of plutonium. Reprocessing/recycling technology has reached maturity in the main nuclear industry countries. Spent fuel reprocessing and recycling of the separated fissile materials remains the main option for the back-end cycle. Today, the operation of MOX-recycling LWRs is considered satisfactory. Experience feedback shows that, in global terms, MOX cores behaviour is equivalent to that of UO 2 cores in terms of operation and safety. (author)

Findings of an international study on burnup credit

International Nuclear Information System (INIS)

Brady, M.C.; Takano, M.; Okuno, H.; DeHart, M.D.; Nouri, A.

1996-01-01

Findings from a four year study by an international benchmarking group in the comparison of computational methods for evaluating burnup credit in criticality safety analyses are presented in this paper. Approximately 20 participants from 11 countries have provided results for most problems. Four detailed benchmark problems for Pressurized Water Reactor (PWR) fuel have been completed and are summarized in this paper. Preliminary results from current work addressing burnup credit for Boiling Water Reactor (BWR) fuel will also be discussed as well as planned activities for additional benchmarks including Mixed-Oxide (MOX) fuels, subcritical benchmarks, international databases, and other activities

Analysis of high burnup fuel safety issues

Energy Technology Data Exchange (ETDEWEB)

Lee, Chan Bock; Kim, D. H.; Bang, J. G.; Kim, Y. M.; Yang, Y. S.; Jung, Y. H.; Jeong, Y. H.; Nam, C.; Baik, J. H.; Song, K. W.; Kim, K. S

2000-12-01

Safety issues in steady state and transient behavior of high burnup LWR fuel above 50 - 60 MWD/kgU were analyzed. Effects of burnup extension upon fuel performance parameters was reviewed, and validity of both the fuel safety criteria and the performance analysis models which were based upon the lower burnup fuel test results was analyzed. It was found that further tests would be necessary in such areas as fuel failure and dispersion for RIA, and high temperature cladding corrosion and mechanical deformation for LOCA. Since domestic fuels have been irradiated in PWR up to burnup higher than 55 MWD/kgU-rod. avg., it can be said that Korea is in the same situation as the other countries in the high burnup fuel safety issues. Therefore, necessary research areas to be performed in Korea were derived. Considering that post-irradiation examination(PIE) for the domestic fuel of burnup higher than 30 MWD/kgU has not been done so far at all, it is primarily necessary to perform PIE for high burnup fuel, and then simulation tests for RIA and LOCA could be performed by using high burnup fuel specimens. For the areas which can not be performed in Korea, international cooperation will be helpful to obtain the test results. With those data base, safety of high burnup domestic fuels will be confirmed, current fuel safety criteria will be re-evaluated, and finally transient high burnup fuel behavior analysis technology will be developed through the fuel performance analysis code development.

Analysis of high burnup fuel safety issues

International Nuclear Information System (INIS)

Lee, Chan Bock; Kim, D. H.; Bang, J. G.; Kim, Y. M.; Yang, Y. S.; Jung, Y. H.; Jeong, Y. H.; Nam, C.; Baik, J. H.; Song, K. W.; Kim, K. S

2000-12-01

Safety issues in steady state and transient behavior of high burnup LWR fuel above 50 - 60 MWD/kgU were analyzed. Effects of burnup extension upon fuel performance parameters was reviewed, and validity of both the fuel safety criteria and the performance analysis models which were based upon the lower burnup fuel test results was analyzed. It was found that further tests would be necessary in such areas as fuel failure and dispersion for RIA, and high temperature cladding corrosion and mechanical deformation for LOCA. Since domestic fuels have been irradiated in PWR up to burnup higher than 55 MWD/kgU-rod. avg., it can be said that Korea is in the same situation as the other countries in the high burnup fuel safety issues. Therefore, necessary research areas to be performed in Korea were derived. Considering that post-irradiation examination(PIE) for the domestic fuel of burnup higher than 30 MWD/kgU has not been done so far at all, it is primarily necessary to perform PIE for high burnup fuel, and then simulation tests for RIA and LOCA could be performed by using high burnup fuel specimens. For the areas which can not be performed in Korea, international cooperation will be helpful to obtain the test results. With those data base, safety of high burnup domestic fuels will be confirmed, current fuel safety criteria will be re-evaluated, and finally transient high burnup fuel behavior analysis technology will be developed through the fuel performance analysis code development

SMOPY, a new NDA tool for safeguards of LEU and MOX spent fuel

International Nuclear Information System (INIS)

Lebrun, A.; Merelli, M.; Szabo, J.-L.; Huver, M.; Arenas-Carrasco, J.

2001-01-01

Upon IAEA request, the French support program to IAEA Safeguards has developed a new device for control of the irradiated LEU and MOX fuels. The Safeguards Mox Python (SMOPY) is the achievement of a 4 years R and D program supported by CEA and COGEMA in partnership with Eurisys Mesures. The SMOPY system is based on the combination of 2 NDA techniques (passive neutron and room temperature gamma spectrometry) and on line interpretation tools (automatic gamma spectrum interpretation, depletion code EVO). Through the measurement managing software, all this contributes to the fully automatic measurement, interpretation and characterization of any kind of spent fuel. The device is transportable (50 kg, 60 cm) and is composed of four parts: 1. the measurement head with one high efficiency fission chamber and a micro room temperature gamma spectrometric probe; 2. the carrier which carries the measurement head. The carrier bottom fits the racks for accurate positioning and its top fits operator's fuel moving tool; 3. the portable electronic cabinet which includes both neutron and gamma electronic cards; 4. the portable PC which gets inspectors data, controls the measurement, get measured values, interprets them and immediately provides the inspector with worthwhile info for appropriate on the field decisions. Main features of SMOPY are: Discrimination of MOX versus LEU irradiated fuels in any case (conservative case is one cycle MOX versus three cycles LEU after short cooling time); Full characterization of irradiated LEU (burnup, cooling time, Pu amounts ...); Partial Defect Test on LEU fuels. A first version of SMOPY has been tested in industrial condition during summer 2000. This tests shown a need of shielding improvement around the gamma detector. A new version has been build a will be qualified during a new field test and then the system will be ready for routine operation in IAEA and commercial delivery. After giving details about the system itself, this paper

Mixed Reload Design Using MOX and UOX Fuel Assemblies

International Nuclear Information System (INIS)

Ramon, Ramirez Sanchez J.; Perry, R.T.

2002-01-01

As part of the studies involved in plutonium utilization assessment for a Boiling Water Reactor, a conceptual design of MOX fuel was developed, this design is mechanically the same design of 10 X 10 BWR fuel assemblies but different fissile material. Several plutonium and gadolinium concentrations were tested to match the 18 months cycle length which is the current cycle length of LVNPP, a reference UO 2 assembly was modeled to have a full cycle length to compare results, an effective value of 0.97 for the multiplication factor was set as target for 470 Effective Full Power days for both cycles, here the gadolinium concentration was a key to find an average fissile plutonium content of 6.55% in the assembly. A reload of 124 fuel assemblies was assumed to simulate the complete core, several load fractions of MOX fuel mixed with UO 2 fresh fuel were tested to verify the shutdown margin, the UO 2 fuel meets the shutdown margin when 124 fuel assemblies are loaded into the core, but it does not happen when those 124 assemblies are replaced with MOX fuel assemblies, so the fraction of MOX was reduced step by step up to find a mixed load that meets both length cycle and shutdown margin. Finally the conclusion is that control rods losses some of their worth in presence of plutonium due to a more hardened neutron spectrum in MOX fuel and this fact limits the load of MOX fuel assemblies in the core, this results are shown in this paper. (authors)

Isotopic Details of the Spent Catawba-1 MOX Fuel Rods at ORNL

Energy Technology Data Exchange (ETDEWEB)

Ellis, Ronald James [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

2015-04-01

The United States Department of Energy funded Shaw/AREVA MOX Services LLC to fabricate four MOX Lead Test Assemblies (LTA) from weapons-grade plutonium. A total of four MOX LTAs (including MX03) were irradiated in the Catawba Nuclear Station (Unit 1) Catawba-1 PWR which operated at a total thermal power of 3411 MWt and had a core with 193 total fuel assemblies. The MOX LTAs were irradiated along with Duke Energy s irradiation of eight Westinghouse Next Generation Fuel (NGF) LEU LTAs (ref.1) and the remaining 181 LEU fuel assemblies. The MX03 LTA was irradiated in the Catawba-1 PWR core (refs.2,3) during cycles C-16 and C-17. C-16 began on June 5, 2005, and ended on November 11, 2006, after 499 effective full power days (EFPDs). C-17 started on December 29, 2006, (after a shutdown of 48 days) and continued for 485 EFPDs. The MX03 and three other MOX LTAs (and other fuel assemblies) were discharged at the end of C-17 on May 3, 2008. The design of the MOX LTAs was based on the (Framatome ANP, Inc.) Mark-BW/MOX1 17 17 fuel assembly design (refs. 4,5,6) for use in Westinghouse PWRs, but with MOX fuel rods with three Pu loading ranges: the nominal Pu loadings are 4.94 wt%, 3.30 wt%, and 2.40 wt%, respectively, for high, medium, and low Pu content. The Mark-BW/MOX1 (MOX LTA) fuel assembly design is the same as the Advanced Mark-BW fuel assembly design but with the LEU fuel rods replaced by MOX fuel rods (ref. 5). The fabrication of the fuel pellets and fuel rods for the MOX LTAs was performed at the Cadarache facility in France, with the fabrication of the LTAs performed at the MELOX facility, also in France.

Fuel component of electricity generation cost for the BN-800 reactor with 800 MOX fuel and uranium oxide fuel, increased fuel burnup, and removal of radial breeding blanket

International Nuclear Information System (INIS)

Raskach, A.

2000-01-01

There are two completed design concepts of NPP with BN-800 type reactors developed with due regard for enhanced safety requirements. They have been created for the 3 rd unit of Beloyarsk NPP and for three units of South Ural NPP. Both concepts are proposed to use mixed oxide fuel (MOX) based on civil plutonium. At this moment economical estimations carried out for these projects need to be revised in connection with the changes of economical situation in Russia and the world nuclear market structure. It is also essential to take into account the existing problem of the excess ex-weapons plutonium utilization and the possibility of using this plutonium to fabricate MOX fuel for the BN-800 reactors. (authors)

Reactors as a Source of Antineutrinos: Effects of Fuel Loading and Burnup for Mixed-Oxide Fuels

Science.gov (United States)

Bernstein, Adam; Bowden, Nathaniel S.; Erickson, Anna S.

2018-01-01

In a conventional light-water reactor loaded with a range of uranium and plutonium-based fuel mixtures, the variation in antineutrino production over the cycle reflects both the initial core fissile inventory and its evolution. Under an assumption of constant thermal power, we calculate the rate at which antineutrinos are emitted from variously fueled cores, and the evolution of that rate as measured by a representative ton-scale antineutrino detector. We find that antineutrino flux decreases with burnup for low-enriched uranium cores, increases for full mixed-oxide (MOX) cores, and does not appreciably change for cores with a MOX fraction of approximately 75%. Accounting for uncertainties in the fission yields in the emitted antineutrino spectra and the detector response function, we show that the difference in corewide MOX fractions at least as small as 8% can be distinguished using a hypothesis test. The test compares the evolution of the antineutrino rate relative to an initial value over part or all of the cycle. The use of relative rates reduces the sensitivity of the test to an independent thermal power measurement, making the result more robust against possible countermeasures. This rate-only approach also offers the potential advantage of reducing the cost and complexity of the antineutrino detectors used to verify the diversion, compared to methods that depend on the use of the antineutrino spectrum. A possible application is the verification of the disposition of surplus plutonium in nuclear reactors.

Increased burnup of fuel elements

International Nuclear Information System (INIS)

Ahlf, J.

1983-01-01

The specialists' group for fuel elements of the Kerntechnische Gesellschaft e.V. held a meeting on ''Increased Burnup of Fuel Elements'' on 9th and 10th of November 1982 at the GKSS Research Center Geesthacht. Most papers dealt with the problems of burnup increase of fuel elements for light water reactors with respect to fuel manufacturing, power plant operation and reprocessing. Review papers were given on the burnup limits for high temperature gas cooled reactors and sodium fast breeder reactors. The meeting ended with a presentation of the technical equipment of the hot laboratory of the GKSS and the programs which are in progress there. (orig.) [de

MOX-fuel inherent proliferation-protection due to {sup 231}Pa admixture

Energy Technology Data Exchange (ETDEWEB)

Kryuchkov, E.F.; Glebov, V.B.; Apse, V.A.; Shmelev, A.N. [Moscow Engineering Physics Institute (State University), Moscow (Russian Federation)

2003-07-01

The proliferation protection levels of MOX-fuel containing small additions of protactinium are evaluated for equilibrium closed and open cycles of a light-water reactor (LWR).Analysis of the ways to the proliferation protection of MOX-fuel by small {sup 231}Pa addition and comparison of this way with another options for giving MOX-fuel the proliferation self-protection property enable us to make the 3 following conclusions: -1) Unique nature of protactinium as a small addition to MOX-fuel is determined by the following properties: - Protactinium is available in the nature (uranium ore) as a long-lived mono-isotope {sup 231}Pa, - under neutron irradiation, {sup 231}Pa is converted into {sup 232}U, which is a long-term source of high energy gamma-radiation and practically non-separable from main fuel mass, - essentially, {sup 231}Pa is a high-quality burnable neutron absorber. -2) From the proliferation self-protection point of view, nuclear fuel cycle closure with fuel recycle is a preferable option because, under this condition, introduction of protactinium into MOX-fuel allows to create the inherent radiation barrier which is in action during full cycle of fuel management at the level corresponding to the accepted today criterion of the Spent Fuel Standard (SFS). In particular, the considered example of multiple MOX-fuel recycle with small addition of {sup 231}Pa (0.2% HM) at each cycle demonstrates a possibility to reach the proliferation protection level of fresh MOX-fuel corresponding to once irradiated fuel with the same cooling time. In this case, the lethal dose (at 30 cm distance from fuel assembly) is received within the minute range. -3) Introduction of {sup 231}Pa into MOX-fuel composition in amount of 0.5% HM allows to prolong action of the SFS from 100 to 200 years. If {sup 231}Pa content is increased up to 5% HM, then MOX-fuel conserves the proliferation self-protection property in respect to short-term unauthorized actions for 200-year period of its

MOX fuel use as a back-end option: Trends, main issues and impacts on fuel cycle management

International Nuclear Information System (INIS)

Fukuda, K.; Choi, J.-S.; Shani, R.; Durpel, L. van den; Bertel, E.; Sartori, E.

2000-01-01

In the past decades while the FBIULWR fuel cycle concept was zealously being developed, MOX-fuel use in thermal reactors was taken as an alternative back-end policy option. However, the plutonium recycling with LWRs has evolved to industrial level, gaining high maturity through the incubative period while FBR deployment was envisaged. Today, MOX-fuel use in LWRs makes integral part of the fuel cycle for those countries relying on the recycling policy. Developments to improve the fuel cycle performance, including the minimisation of remaining wastes, and the reactor engineering aspects owing to MOX-fuel use, are continued. This paper jointly presented by IAEA and OECD/NEA brings an integrated overview on MOX use as a back-end policy, covering MOX fuel utilisation, fuel performance and technology, economics, licensing, MOX fuel trends in the coming decades. (author)

Memento. Maritime transport of MOX fuels from Europe to Japan

International Nuclear Information System (INIS)

1999-07-01

The maritime transport of MOX fuels from Europe to Japan represents the last of the 3 steps of transport of the nuclear fuel reprocessing-recycling program settled between ORC (Japan), BNFL (UK) and Cogema (France). This document summarizes the different aspects of this program: the companies concerned, the physical protection measures, the US-Japan agreements (accompanying warship), the in-depth safety, the handling of MOX fuels (containers and ships), and the Japan MOX fuel needs. (J.S.)

Design of the MOX fuel fabrication facility

International Nuclear Information System (INIS)

Johnson, J.V.; Brabazon, E.J.

2001-01-01

A consortium of Duke Engineering and Services, Inc., COGEMA, Inc. and Stone and Webster (DCS) are designing a mixed oxide fuel fabrication facility (MFFF) for the U.S. Department of Energy (DOE) to convert surplus plutonium to mixed oxide (MOX) fuel to be irradiated in commercial nuclear power plants based on the proven European technology of COGEMA and BELGONUCLEAIRE. This paper describes the MFFF processes, and how the proven MOX fuel fabrication technology is being adapted as required to comply with U.S. requirements. (author)

Design of the MOX fuel fabrication facility

Energy Technology Data Exchange (ETDEWEB)

Johnson, J.V. [MFFF Technical Manager, U.S. dept. of Energy, Washington, DC (United States); Brabazon, E.J. [MFFF Engineering Manager, Duke Cogema Stone and Webster, Charlotte, NC (United States)

2001-07-01

A consortium of Duke Engineering and Services, Inc., COGEMA, Inc. and Stone and Webster (DCS) are designing a mixed oxide fuel fabrication facility (MFFF) for the U.S. Department of Energy (DOE) to convert surplus plutonium to mixed oxide (MOX) fuel to be irradiated in commercial nuclear power plants based on the proven European technology of COGEMA and BELGONUCLEAIRE. This paper describes the MFFF processes, and how the proven MOX fuel fabrication technology is being adapted as required to comply with U.S. requirements. (author)

Comparison of scale/triton and helios burnup calculations for high burnup LWR fuel

Energy Technology Data Exchange (ETDEWEB)

Tittelbach, S.; Mispagel, T.; Phlippen, P.W. [WTI Wissenschaftlich-Technische Ingenieurberatung GmbH, Juelich (Germany)

2009-07-01

The presented analyses provide information about the suitability of the lattice burnup code HELIOS and the recently developed code SCALE/TRITON for the prediction of isotopic compositions of high burnup LWR fuel. The accurate prediction of the isotopic inventory of high burnt spent fuel is a prerequisite for safety analyses in and outside of the reactor core, safe loading of spent fuel into storage casks, design of next generation spent fuel casks and for any consideration of burnup credit. Depletion analyses are performed with both burnup codes for PWR and BWR fuel samples which were irradiated far beyond 50 GWd/t within the LWR-PROTEUS Phase II project. (orig.)

Dissolution behavior of PFBR MOX fuel in nitric acid

International Nuclear Information System (INIS)

Kelkar, Anoop; Kapoor, Y.S.; Singh, Mamta; Meena, D.L.; Pandey, Ashish; Bhatt, R.B.; Behere, P.G.

2017-01-01

Present paper describes the dissolution characteristics of PFBR MOX fuel (U,Pu)O 2 in nitric acid. An overview of batch dissolution experiments, studying the percentage dissolution of uranium and plutonium in (U, Pu)O 2 MOX sintered pellets with different percentage of PuO 2 with reference to time and nitric acid concentration are described. 90% of uranium and plutonium of PFBR MOX gets dissolves in 2 hrs and amount of residue increases with the decrease in nitric acid concentration. Overall variation in percentage residue in PFBR MOX fuel after dissolution test also described. (author)

Technological and licensing challenges for high burnup fuel

International Nuclear Information System (INIS)

Gross, H.; Urban, P.; Fenzlein, C.

2002-01-01

Deregulation of electricity markets is driving electricity prices downward as well in the U.S. as in Europe. As a consequence high burnup fuel will be demanded by utilities using either the storage or the reprocessing option. At a minimum, burnups consistent with the current political enrichment limit of 5 w/o will be required for both markets.Significant progress has been achieved in the past by Siemens in meeting the demands of utilities for increased fuel burnup. The technological challenges posed by the increased burnup are mainly related to the corrosion and hydrogen pickup of the clad, the high burnup properties of the fuel and the dimensional changes of the fuel assembly structure. Clad materials with increased corrosion resistance appropriate for high burnup have been developed. The high burnup behaviour of the fuel has been extensively investigated and the decrease of thermal conductivity with burnup, the rim effect of the pellet and the increase of fission gas release with burnup can be described, with good accuracy, in fuel rod computer codes. Advanced statistical design methods have been developed and introduced. Materials with increased corrosion resistance are also helpful controlling the dimensional changes of the fuel assembly structure. In summary, most of the questions about the fuel operational behaviour and reliability in the high burnup range have been solved - some of them are still in the process of verification - or the solutions are visible. This fact is largely acknowledged by regulators too. The main licensing challenges for high burnup fuel are currently seen for accident condition analyses, especially for RIA and LOCA. (author)

Studies of Flexible MOX/LEU Fuel Cycles

International Nuclear Information System (INIS)

Adams, M.L.; Alonso-Vargas, G.

1999-01-01

This project was a collaborative effort involving researchers from Oak Ridge National Laboratory and North Carolina State University as well as Texas A and M University. The background, briefly, is that the US is planning to use some of its excess weapons Plutonium (Pu) to make mixed-oxide (MOX) fuel for existing light-water reactors (LWRs). Considerable effort has already gone into designing fuel assemblies and core loading patterns for the transition from full-uranium cores to partial-MOX and full-MOX cores. However, these designs have assumed that any time a reactor needs MOX assemblies, these assemblies will be supplied. In reality there are many possible scenarios under which this supply could be disrupted. It therefore seems prudent to verify that a reactor-based Pu-disposition program could tolerate such interruptions in an acceptable manner. Such verification was the overall aim of this project. The task assigned to the Texas A and M team was to use the HELIOS code to develop libraries of two-group homogenized cross sections for the various assembly designs that might be used in a Westinghouse Pressurized Water Reactor (PWR) that is burning weapons-grade MOX fuel. The NCSU team used these cross sections to develop optimized loading patterns under several assumed scenarios. Their results are documented in a companion report

Validation study of core analysis methods for full MOX BWR

International Nuclear Information System (INIS)

2013-01-01

JNES has been developing a technical database used in reviewing validation of core analysis methods of LWRs in the coming occasions: (1) confirming the core safety parameters of the initial core (one-third MOX core) through a full MOX core in Oma Nuclear Power Plant, which is under the construction, (2) licensing high-burnup MOX cores in the future and (3) reviewing topical reports on core analysis codes for safety design and evaluation. Based on the technical database, JNES will issue a guide of reviewing the core analysis methods used for safety design and evaluation of LWRs. The database will be also used for validation and improving of core analysis codes developed by JNES. JNES has progressed with the projects: (1) improving a Doppler reactivity analysis model in a Monte Carlo calculation code MVP, (2) sensitivity study of nuclear cross section date on reactivity calculation of experimental cores composed of UO 2 and MOX fuel rods, (3) analysis of isotopic composition data for UO 2 and MOX fuels and (4) the guide of reviewing the core analysis codes and others. (author)

Validation study of core analysis methods for full MOX BWR

Energy Technology Data Exchange (ETDEWEB)

NONE

2013-08-15

JNES has been developing a technical database used in reviewing validation of core analysis methods of LWRs in the coming occasions: (1) confirming the core safety parameters of the initial core (one-third MOX core) through a full MOX core in Oma Nuclear Power Plant, which is under the construction, (2) licensing high-burnup MOX cores in the future and (3) reviewing topical reports on core analysis codes for safety design and evaluation. Based on the technical database, JNES will issue a guide of reviewing the core analysis methods used for safety design and evaluation of LWRs. The database will be also used for validation and improving of core analysis codes developed by JNES. JNES has progressed with the projects: (1) improving a Doppler reactivity analysis model in a Monte Carlo calculation code MVP, (2) sensitivity study of nuclear cross section date on reactivity calculation of experimental cores composed of UO{sub 2} and MOX fuel rods, (3) analysis of isotopic composition data for UO{sub 2} and MOX fuels and (4) the guide of reviewing the core analysis codes and others. (author)

Use of destructive and nondestructive methods of analysis for quality assurance at MOX fuel production in the Russia

International Nuclear Information System (INIS)

Bibilashvili, Y.K.; Rudenko, V.S.; Chorokhov, N.A.; Korovin, Y.I.; Petrov, A.M.; Vorobiev, A.V.; Mukhortov, N.F.; Smirnov, Y.A.; Kudryavtsev, V.N.

2000-01-01

Parameters of MOX fuel with various plutonium contents are considered from the point of view of necessity of their control for quality assurance. Destructive and nondestructive methods used for this purpose in the Russia are described: controlled potential coulometry for determination of uranium or/and plutonium contents, their ratio and oxygen factor; mass spectrometry for determination of uranium and plutonium isotopic composition; chemical spectral emission method for determination of contents of 'metal' impurities, boron and silicon, and methods of determination of gas forming impurities. Capabilities of nondestructive gamma-ray spectrometry techniques are considered in detail and results of their use at measurement of uranium and plutonium isotopic composition in initial dioxides, at determination of contents of uranium and plutonium, and uniformity of their distribution in MOX powder and pellets. The necessity of correction of algorithm of the MGA program is shown for using the program at analyses of gamma-ray spectra of MOX with low contents of low burnup plutonium. (authors)

Physical models for high burnup fuel

International Nuclear Information System (INIS)

Kanyukova, V.; Khoruzhii, O.; Likhanskii, V.; Solodovnikov, G.; Sorokin, A.

2003-01-01

In this paper some models of processes in high burnup fuel developed in Src of Russia Troitsk Institute for Innovation and Fusion Research are presented. The emphasis is on the description of the degradation of the fuel heat conductivity, radial profiles of the burnup and the plutonium accumulation, restructuring of the pellet rim, mechanical pellet-cladding interaction. The results demonstrate the possibility of rather accurate description of the behaviour of the fuel of high burnup on the base of simplified models in frame of the fuel performance code if the models are physically ground. The development of such models requires the performance of the detailed physical analysis to serve as a test for a correct choice of allowable simplifications. This approach was applied in the SRC of Russia TRINITI to develop a set of models for the WWER fuel resulting in high reliability of predictions in simulation of the high burnup fuel

Validation of MOX fuel through recent BELGONUCLEAIRE international programmes

International Nuclear Information System (INIS)

Basselier, J.; Maldague, T.; Lippens, M.

1997-01-01

The paper reviews the present experience of BELGONUCLEAIRE in promoting and managing international programmes dedicated to improvement and updating of MOX fuel data bases on what concerns core physics and rod behaviour with a view of assist all MOX fuel designers and users in their validation and modelization work. All these programmes were completed or will be completed with the support of numerous international organizations deeply concerned by MOX recycling strategies. (author). 9 figs, 2 tabs

Experimental microstructures MOX fuels elaboration

International Nuclear Information System (INIS)

Gotta, M.J.; Dubois, S.; Lechelle, J.; Sornay, P.

2000-01-01

In order to propose a new MOX fuel, owning higher combustion rate, studies are realized at the CEA in collaboration with Cogema, EDF and Framatome. New microstructures of MOX are looked for around two approaches: the grains size and the plutonium distribution. These approaches are presented and discussed in this paper. The first one develops big grains microstructures obtained, either with anionic (sulfur), or cationic (Cr 2 O 3 ) additives. The second one concerns the CER-CER type composite microstructures. (A.L.B.)

Power ramp tests of MOX fuel rods. HBWR irradiation with the instrument rig, IFA-591

International Nuclear Information System (INIS)

Ozawa, Takayuki; Abe, Tomoyuki

2006-03-01

Plutonium-uranium mixed oxide (MOX) fuel rods of instrumental rig IFA-591 were ramped in HBWR to study the Advanced Thermal Reactor (ATR) MOX fuel behavior during transient operation and to determine a failure threshold of the MOX fuel rods. Eleven segments were base-irradiated in ATR 'FUGEN' up to 18.4 GWd/t. Zirconium liner claddings were adopted for four segments of them. As the results of non-destructive post irradiation examinations (PIEs) after the base-irradiation and before the ramp tests, no remarkable behavior affecting the integrity of fuel assembly and fuel rod was confirmed. All segments to be used for the ramp tests, which consisted of the multi-step ramp tests and the single-step ramp tests, had instrumentations for in-pile measurements of cladding elongation or plenum pressure, and heated up to the maximum linear power of 58.3-68.4 kW/m without failure. The major results of ramp tests are as follows: There is no difference in PCMI behaviors between two type rods of Zry-2 and Zirconium liner claddings from the in-pile measurements of cladding elongation and plenum pressure. The computations of cladding elongation and inner pressure gave slightly lower elongation and pressure than the in-pile measurements during the ramp-test. However, the cladding relaxation during the power hold was in good agreement, and the fission gas release behavior during cooling down could be evaluated by taking into account the relaxation of contact pressure between pellet and cladding. Although the final power during IFA-591 ramp tests reached the higher linear power than the failure threshold power of UO 2 fuel rods, no indication of fuel failure was observed during the ramp tests. The cladding relaxation due to the creep deformation of the MOX pellets at high temperature could be confirmed at the power steps during the multi-ramp test. The fission gas release due to the emancipation from PCMI stress was observed during the power decreasing. The burn-up dependence could be

Development of high burnup nuclear fuel technology

International Nuclear Information System (INIS)

Suk, Ho Chun; Kang, Young Hwan; Jung, Jin Gone; Hwang, Won; Park, Zoo Hwan; Ryu, Woo Seog; Kim, Bong Goo; Kim, Il Gone

1987-04-01

The objectives of the project are mainly to develope both design and manufacturing technologies for 600 MWe-CANDU-PHWR-type high burnup nuclear fuel, and secondly to build up the foundation of PWR high burnup nuclear fuel technology on the basis of KAERI technology localized upon the standard 600 MWe-CANDU- PHWR nuclear fuel. So, as in the first stage, the goal of the program in the last one year was set up mainly to establish the concept of the nuclear fuel pellet design and manufacturing. The economic incentives for high burnup nuclear fuel technology development are improvement of fuel utilization, backend costs plant operation, etc. Forming the most important incentives of fuel cycle costs reduction and improvement of power operation, etc., the development of high burnup nuclear fuel technology and also the research on the incore fuel management and safety and technologies are necessary in this country

Verification of spectral burn-up codes on 2D fuel assemblies of the GFR demonstrator ALLEGRO reactor

International Nuclear Information System (INIS)

Čerba, Štefan; Vrban, Branislav; Lüley, Jakub; Dařílek, Petr; Zajac, Radoslav; Nečas, Vladimír; Haščik, Ján

2014-01-01

Highlights: • Verification of the MCNPX, HELIOS and SCALE codes. • MOX and ceramic fuel assembly. • Gas-cooled fast reactor. • Burnup calculation. - Abstract: The gas-cooled fast reactor, which is one of the six GEN IV reactor concepts, is characterized by high operational temperatures and a hard neutron spectrum. The utilization of commonly used spectral codes, developed mainly for LWR reactors operated in the thermal/epithermal neutron spectrum, may be connected with systematic deviations since the main development effort of these codes has been focused on the thermal part of the neutron spectrum. To be able to carry out proper calculations for fast systems the used codes have to account for neutron resonances including the self-shielding effect. The presented study aims at verifying the spectral HELIOS, MCNPX and SCALE codes on the basis of depletion calculations of 2D MOX and ceramic fuel assemblies of the ALLEGRO gas-cooled fast reactor demonstrator in infinite lattice

The applicability of detailed process for neutron resonance absorption to neutronics analyses in LWR next generation fuels to extend burnup

International Nuclear Information System (INIS)

Kameyama, Takanori; Nauchi, Yasushi

2004-01-01

Neutronics analyses with detail processing for neutron resonance absorption in LWR next generation UOX and MOX fuels to extend burnup were performed based on the neutronic transport and burnup calculation. In the detailed processing, ultra-fine energy nuclear library and collision probabilities between neutron and U, Pu nuclides (actinide nuclides) are utilized for two-dimension geometry. In the usual simple processing (narrow resonance approximation), shielding factors and compensation equations for neutron resonance absorption are utilized. The results with detailed and simple processing were compared to clarify where the detailed processing is needed. The two processing caused difference of neutron multiplication factor by 0.5% at the beginning of irradiation, while the difference became smaller as burnup increased and was not significant at high burnup. The nuclide compositions of the fuel rods for main actinide nuclides were little different besides Cm isotopes by the processing, since the neutron absorption rate of 244 Cm became different. The detail processing is needed to evaluate the neutron emission rate in spent fuels. In the fuel assemblies, the distributions of rod power rates were not different within 0.5%, and the peak rates of fuel rod were almost the same by the two processing at the beginning of irradiation when the peak rate is the largest during the irradiation. The simple processing is also satisfied for safety evaluation based on the peak rate of rod power. The difference of local power densities in fuel pellets became larger as burnup increased, since the neutron absorption rate of 238 U in the peripheral region of pellets were significantly different by the two processing. The detail processing is needed to evaluate the fuel behavior at high burnup. (author)

A risk-informed evaluation of MOX fuel loading in PWRS

International Nuclear Information System (INIS)

Lyman, E.S.

2001-01-01

The full text follows: The U.S. Department of Energy (DOE) has signed a contract with Duke Cogema Stone and Webster (DCS) for fabrication of mixed-oxide (MOX) fuel and irradiation of the MOX fuel at the Catawba and McGuire pressurized-water reactors (PWRs), operated by Duke Power. The first load of MOX fuel is scheduled for 2007. In order to use MOX in these plants, Duke Power will have to apply to the Nuclear Regulatory Commission (NRC) for amendments to their operating licenses. Until recently, there have been no numerical guidelines for determining the acceptability of license amendment requests. However, such guidelines are now at hand with the adoption in 1998 of NRC Regulatory Guide 1.174, which defines a maximum value for the permissible increase in risk to the public resulting from a proposed change to a nuclear plant's licensing basis (LB). The substitution of MOX fuel for low-enriched uranium (LEU) fuel in LWRs will have an impact on risk to the public that will require regulatory evaluation. One of the major differences is that use of MOX will increase the inventories of plutonium and minor actinides in the reactor core, thereby increasing the source term for certain severe accidents, such as a core melt with early containment failure or a spent fuel pool drain-down. The goal of this paper is to quantitatively evaluate the increase in risk associated with the greater actinide source term in MOX-fueled reactors, and to compare this increase with RG 1.174 guidelines. Standard computer programs (SCALE and MACCS2) are used to estimate the increase in severe accident risk to the public associated with the DCS plan to use 40% cores of weapons-grade MOX fuel. These values are then compared to the RG 1.174 acceptance criteria, using publicly available risk information. Since RG 1.174 guidelines are based on the assumption that severe accident source terms are not affected by LB changes, the RG 1.174 formalism must be modified for this case. A similar

Needs of reliable nuclear data and covariance matrices for Burnup Credit in JEFF-3 library

International Nuclear Information System (INIS)

Chambon, A.; Santamarina, A.; Riffard, C.; Lavaud, F.; Lecarpentier, D.

2013-01-01

Burnup Credit (BUC) is the concept which consists in taking into account credit for the reduction of nuclear spent fuel reactivity due to its burnup. In the case of PWR-MOx spent fuel, studies pointed out that the contribution of the 15 most absorbing, stable and non-volatile fission products selected to the credit is as important as the one of the actinides. In order to get a 'best estimate' value of the keff, biases of their inventory calculation and individual reactivity worth should be considered in criticality safety studies. This paper enhances the most penalizing bias towards criticality and highlights possible improvements of nuclear data for the 15 fission products (FPs) of PWR-MOx BUC. Concerning the fuel inventory, trends in function of the burnup can be derived from experimental validation of the DARWIN-2.3 package (using the JEFF- 3.1.1/SHEM library). Thanks to the BUC oscillation programme of separated FPs in the MINERVE reactor and fully validated scheme PIMS, calculation over experiment ratios can be accurately transposed to tendencies on the FPs integral cross sections. (authors)

The need for integral critical experiments with low-moderated MOX fuels

International Nuclear Information System (INIS)

2004-01-01

The use of MOX fuel in commercial reactors is a means of burning plutonium originating from either surplus weapons or reprocessed irradiated uranium fuel. This requires the fabrication of MOX assemblies on an industrial scale. The OECD/NEA Expert Group on Experimental Needs for Criticality Safety has highlighted MOX fuel manufacturing, as an area in which there is a specific need for additional experimental data for validation purposes. Indeed, integral experiments with low-moderated MOX fuel are either scarce or not sufficiently accurate to provide an appropriate degree of validation of nuclear data and computer codes. New and accurate experimental data would enable a better optimisation of the fabrication process by decreasing the uncertainties in the determination of multiplication factors of configurations such as the homogenization of MOX powders. In this context, the OECD/NEA Nuclear Science Committee organised a workshop to address the following topics: expression and justification of the need for critical or near-critical experiments employing low-moderated MOX fuels; proposals for experimental programmes to address these needs; prospects for an international co-operative programme. The workshop was held at OECD headquarters in Paris on 14-15 April 2004. (author)

The feasibility study on fuel types for the KALIMER

International Nuclear Information System (INIS)

Hwang, W.; Nam, C.; Yim, J. S.; Na, B. C.; Hahn, D. H.; Kim, Y. I.; Kim, Y. C.; Park, C. K.

1997-08-01

The economics of LMR is largely dependent on the construction cost of the power plant, and the fuel cycle options usually constitute 20 to 30 % of total electricity generation cost. The choice of fuel cycle technology and the fuel type is important in order to develop a LMR with better economics, performance and safety. The LMR fuel types, whose performances have been proven up to 15 at% burnup, are MOX and IFR metal fuel. The base alloy, binary (U-10% Zr) metal fuel with HT9 is used as structural materials of KALIMER. The design concept of KALIMER fuel has been established through the investigation of technical feasibilities on the fuel and recycle systems for MOX and IFR metal fuel. According to the results of comparative analysis for MOX and metal fuel, metal fuel is better than MOX in view of safety, in-reactor performance, nuclear characteristics, economics and non-proliferation, while MOX fuels have advantages in the developmental status and technical cooperation potential. The overall performance of binary (U-10% Zr) metal fuel with HT9 cladding, which is a potential start-up fuel for KALIMER, is not only superior to that of MOX fuel, but also has enough technical feasibility in its high-burnup performance, safety and economics. (author). 54 ref., 13 tabs., 20 figs

Safety analysis of MOX fuels by fuel performance code

Energy Technology Data Exchange (ETDEWEB)

Suzuki, Motoe [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

2002-12-01

Performance of plutonium rick mixed oxide fuels specified for the Reduced-Moderation Water Reactor (RMWR) has been analysed by modified fuel performance code. Thermodynamic properties of these fuels up to 120 GWd/t burnup have not been measured and estimated using existing uranium fuel models. Fission product release, pressure rise inside fuel rods and mechanical loads of fuel cans due to internal pressure have been preliminarily assessed based on assumed axial power distribution history, which show the integrity of fuel performance. Detailed evaluation of fuel-cladding interactions due to thermal expansion or swelling of fuel pellets due to high burnup will be required for safety analysis of mixed oxide fuels. Thermal conductivity and swelling of plutonium rich mixed oxide fuels shall be taken into consideration. (T. Tanaka)

Safety-related investigations on power distribution in MOX fuel elements in LWR cores

International Nuclear Information System (INIS)

Kramer, E.; Langenbuch, S.

1991-01-01

For the concept of thermal recycling various fuel assembly designs have been developped during the last years. An overview is given describing the present status of MOX-fuel assembly design for PWR and BWR. The local power distribution within the MOX-fuel assembly and influences between neighbouring MOX- and Uranium fuel assemblies have been analyzed by own calculations. These investigations are limited to specific aspects of the spatial power distribution, which are related to the use of MOX-fuel assemblies within the reactor core of LWR. (orig.) [de

An evaluation of the deployment of AIROX-recycled fuel in pressurized water reactors

International Nuclear Information System (INIS)

Jahshan, S.N.; McGeehan, T.J.

1994-01-01

An analytical evaluation is made of the pressurized water reactor (PWR) in-core performance of recycled light water reactor fuel that has been Atomics International reduction oxidation (AIROX) reprocessed and reenriched with fissile materials. The neutronics performance is shown to lie within the neutronics performance of existing high-performance and high-burnup fuels. Three AIROX-recycled fuels are compared with a high-burnup virgin fuel and an equivalent mixed-oxide (MOX) fuel. The AIROX-recycled fuel neutronics performance lies consistently between the virgin and the MOX fuel for both the pin power peaking and the reactivity response characteristics in PWRs. Among the attractive features of AIROX-recycled fuel is that it can optimize fissile and fertile fuel use, minimize final fuel disposal impact on the environment, and provide energy in the process of denaturing weapons-grade fissile materials. The fuel material performance may be anticipated from high-burnup virgin fuel and from MOX fuel performance. Recommendations for lead rod testing and for optimization of the AIROX-processing and resintering techniques are made

Nuclear fuel burn-up economy

International Nuclear Information System (INIS)

Matausek, M.

1984-01-01

In the period 1981-1985, for the needs of Utility Organization, Beograd, and with the support of the Scientific Council of SR Srbija, work has been performed on the study entitled 'Nuclear Fuel Burn-up Economy'. The forst [phase, completed during the year 1983 comprised: comparative analysis of commercial NPP from the standpoint of nuclear fuel requirements; development of methods for fuel burn-up analysis; specification of elements concerning the nuclear fuel for the tender documentation. The present paper gives the short description of the purpose, content and results achieved in the up-to-now work on the study. (author)

Assessment of dry storage performance of spent LWR fuel assemblies with increasing burnup

International Nuclear Information System (INIS)

Peehs, M.; Garzarolli, F.; Goll, W.

1999-01-01

Although the safety of a dry long-term spent fuel store is scarcely influenced if a few fuel rods start to leak during extended storage - since all confinement systems are designed to retain gaseous activity safely - it is a very conservative safety goal to avoid the occurrence of systematic rod defects. To assess the extended storage performance of a spent fuel assembly (FA), the experience can be collated into 3 storage modes: I - fast rate of temperature decrease δ max ≥ δ ≥ 300 deg. C, II - medium rate of decrease for the fuel rod dry storage temperature 300 deg. C > δ ≥ 200 deg. C, III - slow to negligible rate of temperature decrease for δ 2 -fuel are practically immobile during storage. Consequently all fission-product-driven defect mechanisms will not take place. The leading defect mechanism - also for fuel rods with increased burnup - remains creep due to the hoop strain resulting from the fuel rod internal fission gas pressure. Limiting the creep to its primary and secondary stages prevents fuel rod degradation. The allowable uniform strain of the cladding is 1 - 2%. Calculations were performed to predict the dry storage performance of fuel assemblies with a burnup ≤ 55 GW · d/tHM based on the fuel assemblies end of life (EOL)-data and on a representative curve T = f(t). The maximum allowable hot spot temperature of a fuel rod in the CASTOR V cask was between 348 deg. C (U FA) and 358 deg. C (MOX FA). The highest hoop strain predicted after 40 years of storage is 0.77% proving that spent LWR fuel dry storage is safe. (author)

Advanced high throughput MOX fuel fabrication technology and sustainable development

International Nuclear Information System (INIS)

Krellmann, Juergen

2005-01-01

The MELOX plant in the south of France together with the La Hague reprocessing plant, are part of the two industrial facilities in charge of closing the nuclear fuel cycle in France. Started up in 1995, MELOX has since accumulated a solid know-how in recycling plutonium recovered from spent uranium fuel into MOX: a fuel blend comprised of both uranium and plutonium oxides. Converting recovered Pu into a proliferation-resistant material that can readily be used to power a civil nuclear reactor, MOX fabrication offers a sustainable solution to safely take advantage of the plutonium's high energy content. Being the first large-capacity industrial facility dedicated to MOX fuel fabrication, MELOX distinguishes itself from the first generation MOX plants with high capacity (around 200 tHM versus around 40 tHM) and several unique operational features designed to improve productivity, reliability and flexibility while maintaining high safety standards. Providing an exemplary reference for high throughput MOX fabrication with 1,000 tHM produced since start-up, the unique process and technologies implemented at MELOX are currently inspiring other MOX plant construction projects (in Japan with the J-MOX plant, in the US and in Russia as part of the weapon-grade plutonium inventory reduction). Spurred by the growing international demand, MELOX has embarked upon an ambitious production development and diversification plan. Starting from an annual level of 100 tons of heavy metal (tHM), MELOX demonstrated production capacity is continuously increasing: MELOX is now aiming for a minimum of 140 tHM by the end of 2005, with the ultimate ambition of reaching the full capacity of the plant (around 200 tHM) in the near future. With regards to its activity, MELOX also remains deeply committed to sustainable development in a consolidated involvement within AREVA group. The French minister of Industry, on August 26th 2005, acknowledged the benefits of MOX fuel production at MELOX: 'In

A comparative study of fission gas behaviour in UO2 and MOX fuels using the meteor fuel performance code

International Nuclear Information System (INIS)

Struzik, C.; Garcia, Ph.; Noirot, L.

2002-01-01

The paper reviews some of the fission-gas-related differences observed between MOX MIMAS AUC fuels and homogeneous UO 2 fuels. Under steady-state conditions, the apparently higher fractional release in MOX fuels is interpreted with the METEOR fuel performance code as a consequence of their lower thermal conductivity and the higher linear heat rates to which MOX fuel rods are subjected. Although more fundamental diffusion properties are needed, the apparently greater swelling of MOX fuel rods at higher linear heat rates can be ascribed to enhanced diffusion properties. (authors)

A MOX fuel attribute monitor

International Nuclear Information System (INIS)

Bliss, Mary; Jordan, David V.; Barnett, Debra S.; Redding, Rebecca L.; Pearce, Stephen K.

2007-01-01

Euratom performs safeguards monitoring of Fresh MOX fuel for domestic power production in the European Union. Video cameras monitor the reactor storage ponds. If video surveillance is lost for a certain amount of time a measurement is required to verify that no fuel was diverted. The attribute measurement to verify the continued presence of MOX fuel is neutron emission. Ideally this measurement would be made without moving or handling the fuel rod assembly. A prototype attribute measurement system was made using scintillating neutron sensitive glass waveguides developed by Pacific Northwest National Laboratory. Short lengths (5-20 cm) of the neutron sensitive fiber were mechanically spliced to 15 m lengths of commercial high numerical aperture fiber optic cable (Ceramoptec Optran Ultra 0.44). The light detector is a Hamamatsu R7400P photomultiplier tube. An electronics package was built to use the sensors with a GBS Elektronik MCA-166 multichannel analyzer and user interface. The MCA-166 is the system most commonly used by Euratom inspectors. It can also be run from a laptop computer using Maestro (Ortec) or other software. A MCNP model was made to compare to measurements made with several neutron sources including NIST traceable 252 Cf

Fuel cycles with high fuel burn-up: analysis of reactivity coefficients

International Nuclear Information System (INIS)

Kryuchkov, E.F.; Shmelev, A.N.; Ternovykh, M.J.; Tikhomirov, G.V.; Jinhong, L.; Saito, M.

2003-01-01

Fuel cycles of light-water reactors (LWR) with high fuel burn-up (above 100 MWd/kg), as a rule, involve large amounts of fissionable materials. It leads to forming the neutron spectrum harder than that in traditional LWR. Change of neutron spectrum and significant amount of non-traditional isotopes (for example, 237 Np, 238 Pu, 231 Pa, 232 U) in such fuel compositions can alter substantially reactivity coefficients as compared with traditional uranium-based fuel. The present work addresses the fuel cycles with high fuel burn-up which are based on Th-Pa-U and U-Np-Pu fuel compositions. Numerical analyses are carried out to determine effective neutron multiplication factor and void reactivity coefficient (VRC) for different values of fuel burn-up and different lattice parameters. The algorithm is proposed for analysis of isotopes contribution to these coefficients. Various ways are considered to upgrade safety of nuclear fuel cycles with high fuel burn-up. So, the results obtained in this study have demonstrated that: -1) Non-traditional fuel compositions developed for achievement of high fuel burn-up in LWR can possess positive values of reactivity coefficients that is unacceptable from the reactor operation safety point of view; -2) The lattice pitch of traditional LWR is not optimal for non-traditional fuel compositions, the increased value of the lattice pitch leads to larger value of initial reactivity margin and provides negative VRC within sufficiently broad range of coolant density; -3) Fuel burn-up has an insignificant effect on VRC dependence on coolant density, so, the measures undertaken to suppress positive VRC of fresh fuel will be effective for partially burnt-up fuel compositions also and; -4) Increase of LWR core height and introduction of additional moderators into the fuel lattice can be used as the ways to reach negative VRC values for full range of possible coolant density variations

IFPE/CNEA-MOX-RAMP, CNEA Power Ramp Irradiations with (PHWR) MOX Fuels

International Nuclear Information System (INIS)

Marino, Armando Carlos; Turnbull, J.A.

2000-01-01

Description: The irradiation of the first MOX nuclear fuel rods fabricated in Argentina began in 1986. These experiences were made in the HFR-Petten reactor, Holland. The six rods were fabricated in the a Facility (GAID-CNEA-Argentina). The first rod has been used for destructive pre-irradiation characterization in the KFK (Kernforschungszentrum Karlsruhe), Germany. The second one was a pathfinder for calibrating HFR systems in Petten. Two other rods included pellets doped with iodine. The first contained mostly CsI whilst the second contained elemental iodine. The concentration of iodine was intended to simulate a burn-up of 15000 MWd/ton(M). The power histories were defined from calculations performed with the BACO code. A 15 day cycle was assumed with a power history that induced PCMI during power cycling. The last high power period was maintained until stress corrosion cracking (SCC) was induced. Two further un-doped rods were used in a sub-program named BU15. Here a burn-up of 15000 MWd/ton(M) was achieved at a low power followed by a final power ramp for one of the rods. The ramp was similar to that used for the Iodine test. The HFR irradiation was conducted satisfactorily. The objective was to attempt a correspondence in behaviour between the doped rods and BU15 rods. PIE detected the presence of micro-cracks inside the cladding of the iodine doped rods. Ramping of the BU15 rod was interrupted when an increase of coolant activity was detected. After discharge, a visual inspection of the rod showed the presence of a small circular hole in the cladding. Additional PIE showed that the hole was due to a SCC failure

Nuclear fuel activities in Canada

Energy Technology Data Exchange (ETDEWEB)

Cox, D S [Fuel Development Branch, Chalk River Labs., AECL (Canada)

1997-12-01

Nuclear fuel activities in Canada are considered in the presentation on the following directions: Canadian utility fuel performance; CANDU owner`s group fuel programs; AECL advanced fuel program (high burnup fuel behaviour and development); Pu dispositioning (MOX) activities. 1 tab.

Radial power density distribution of MOX fuel rods in the HBWR

International Nuclear Information System (INIS)

Koo, Yang Hyun; Joo, Hyung Kook; Lee, Byung Ho; Sohn, Dong Seong

1999-07-01

Two MOX fuel rods, which ar being fabricated in the Paul Scherrer Institute (PSI), Switzerland in cooperation with the Korea Atomic Energy Research Institute (KAERI), are going to be irradiated in the HBWR (Halden Boiling Water Reactor) from the beginning of 2000 in the framework of OECD Halden Reactor Programme (HRP) together with a reference MOX fuel rod supplied by the BNFL. Since fuel temperature, which is influenced by radial power distribution, is a basic property in analyzing fuel behavior, it is required to consider radial power distribution in the HBWR. A subroutine FACTOR H BWR that calculates radial power density distribution for three MOX fuel rods have been developed subroutine FACTOR H BWR gives good agreement with the physics calculation except slight underprediction in the central part and a little overprediction at the outer part of the pellet. The subroutine will be incorporated into a computer code COSMOS and used to analyze the in-reactor behavior of the three MOX fuel rods during the Halden irradiation test. (author). 5 refs., 3 tabs., 24 figs

Automated generation of burnup chain for reactor analysis applications

International Nuclear Information System (INIS)

Tran, Viet-Phu; Tran, Hoai-Nam; Yamamoto, Akio; Endo, Tomohiro

2017-01-01

This paper presents the development of an automated generation of burnup chain for reactor analysis applications. Algorithms are proposed to reevaluate decay modes, branching ratios and effective fission product (FP) cumulative yields of a given list of important FPs taking into account intermediate reactions. A new burnup chain is generated using the updated data sources taken from the JENDL FP decay data file 2011 and Fission yields data file 2011. The new burnup chain is output according to the format for the SRAC code system. Verification has been performed to evaluate the accuracy of the new burnup chain. The results show that the new burnup chain reproduces well the results of a reference one with 193 fission products used in SRAC. Burnup calculations using the new burnup chain have also been performed based on UO_2 and MOX fuel pin cells and compared with a reference chain th2cm6fp193bp6T.

Automated generation of burnup chain for reactor analysis applications

Energy Technology Data Exchange (ETDEWEB)

Tran, Viet-Phu [VINATOM, Hanoi (Viet Nam). Inst. for Nuclear Science and Technology; Tran, Hoai-Nam [Duy Tan Univ., Da Nang (Viet Nam). Inst. of Research and Development; Yamamoto, Akio; Endo, Tomohiro [Nagoya Univ., Nagoya-shi (Japan). Dept. of Materials, Physics and Energy Engineering

2017-05-15

This paper presents the development of an automated generation of burnup chain for reactor analysis applications. Algorithms are proposed to reevaluate decay modes, branching ratios and effective fission product (FP) cumulative yields of a given list of important FPs taking into account intermediate reactions. A new burnup chain is generated using the updated data sources taken from the JENDL FP decay data file 2011 and Fission yields data file 2011. The new burnup chain is output according to the format for the SRAC code system. Verification has been performed to evaluate the accuracy of the new burnup chain. The results show that the new burnup chain reproduces well the results of a reference one with 193 fission products used in SRAC. Burnup calculations using the new burnup chain have also been performed based on UO{sub 2} and MOX fuel pin cells and compared with a reference chain th2cm6fp193bp6T.

Fuel cycles with high fuel burn-up: analysis of reactivity coefficients

Energy Technology Data Exchange (ETDEWEB)

Kryuchkov, E.F.; Shmelev, A.N.; Ternovykh, M.J.; Tikhomirov, G.V.; Jinhong, L. [Moscow Engineering Physics Institute (State University) (Russian Federation); Saito, M. [Tokyo Institute of Technology (Japan)

2003-07-01

Fuel cycles of light-water reactors (LWR) with high fuel burn-up (above 100 MWd/kg), as a rule, involve large amounts of fissionable materials. It leads to forming the neutron spectrum harder than that in traditional LWR. Change of neutron spectrum and significant amount of non-traditional isotopes (for example, {sup 237}Np, {sup 238}Pu, {sup 231}Pa, {sup 232}U) in such fuel compositions can alter substantially reactivity coefficients as compared with traditional uranium-based fuel. The present work addresses the fuel cycles with high fuel burn-up which are based on Th-Pa-U and U-Np-Pu fuel compositions. Numerical analyses are carried out to determine effective neutron multiplication factor and void reactivity coefficient (VRC) for different values of fuel burn-up and different lattice parameters. The algorithm is proposed for analysis of isotopes contribution to these coefficients. Various ways are considered to upgrade safety of nuclear fuel cycles with high fuel burn-up. So, the results obtained in this study have demonstrated that: -1) Non-traditional fuel compositions developed for achievement of high fuel burn-up in LWR can possess positive values of reactivity coefficients that is unacceptable from the reactor operation safety point of view; -2) The lattice pitch of traditional LWR is not optimal for non-traditional fuel compositions, the increased value of the lattice pitch leads to larger value of initial reactivity margin and provides negative VRC within sufficiently broad range of coolant density; -3) Fuel burn-up has an insignificant effect on VRC dependence on coolant density, so, the measures undertaken to suppress positive VRC of fresh fuel will be effective for partially burnt-up fuel compositions also and; -4) Increase of LWR core height and introduction of additional moderators into the fuel lattice can be used as the ways to reach negative VRC values for full range of possible coolant density variations.

Influence of plutonium contents in MOX fuel on destructive forces at fuel failure in the NSRR experiment

Energy Technology Data Exchange (ETDEWEB)

Nakamura, Jinichi; Sugiyama, Tomoyuki; Nakamura, Takehiko; Kanazawa, Toru; Sasajima, Hideo [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

2003-03-01

In order to confirm safety margins of the Mixed Oxide (MOX) fuel use in LWRs, pulse irradiation tests are planned in the Nuclear Safety Research Reactor (NSRR) with the MOX fuel with plutonium content up to 12.8%. Impacts of the higher plutonium contents on safety of the reactivity-initiated-accident (RIA) tests are examined in terms of generation of destructive forces to threat the integrity of test capsules. Pressure pulses would be generated at fuel rod failure by releases of high pressure gases. The strength of the pressure pulses, therefore, depends on rod internal - external pressure difference, which is independent to plutonium content of the fuel. The other destructive forces, water hammer, would be generated by thermal interaction between fuel fragments and coolant water. Heat flux from the fragments to the water was calculated taking account of changes in thermal properties of MOX fuels at higher plutonium contents. The results showed that the heat transfer from the MOX fuel would be slightly smaller than that from UO{sub 2} fuel fragments at similar size in a short period to cause the water hammer. Therefore, the destructive forces were not expected to increase in the new tests with higher plutonium content MOX fuels. (author)

Some results on development, irradiation and post-irradiation examinations of fuels for fast reactor-actinide burner (MOX and inert matrix fuel)

International Nuclear Information System (INIS)

Poplavsky, V.; Zabudko, L.; Moseev, L.; Rogozkin, B.; Kurina, I.

1996-01-01

Studies performed have shown principal feasibility of the BN-600 and BN-800 cores to achieve high efficiency of Pu burning when MOX fuel with Pu content up to 45% is used. Valuable experience on irradiation behaviour of oxide fuel with high Pu content (100%) was gained as a result of operation of two BR-10 core loadings where the maximum burnup 14 at.% was reached. Post-irradiation examination (PIE) allowed to reveal some specific features of the fuel with high plutonium content. Principal irradiation and PIE results are presented in the paper. Use of new fuel without U-238 provides the maximum burning capability as in this case the conversion ratio is reduced to zero. Technological investigations of inert matrix fuels have been continued now. Zirconium carbide, zirconium nitride, magnesium oxide and other matrix materials are under consideration. Inert matrices selection criteria are discussed in the paper. Results of technological study, of irradiation in the BOR-60 reactor and PIE results of some inert matrix fuels are summarized in this report. (author). 2 refs, 1 fig., 3 tabs

Recent prospects of MOX fuel and strategy about nuclear fuel cycle

International Nuclear Information System (INIS)

Liu Dingqin

1991-04-01

It is clearly described what is the preliminary adequate strategic concern for different nuclear power countries under different nuclear power development conditions. It is also stressed on the basic situation of the design technology, manufacture technology, operation experiences and quantitative economic analysis for MOX fuel application since fast breed reactor commercialization has been delayed. The author specially proposed that in a short term China should adopt an intermediate storage strategy matched with the construction of a pilot reprocessing plant to prepare the technical basis for commercialized reprocessing plant later on and to follow the development of MOX fuel technology

A programmatic approach for implementing MOX fuel operation in advanced and existing boiling water reactors

International Nuclear Information System (INIS)

Ehrlich, E.H.; Knecht, P.D.; Shirley, N.C.; Wadekamper, D.C.

1996-01-01

This paper describes a programmatic overview of the elements and issues associated with MOX fuel utilization. Many of the dominant considerations and integrated relationships inherent in initiating MOX fuel utilization in BWRs or the ABWR with partial or full MOX core designs are discussed. The most significant considerations in carrying out a MOX implementation program, while achieving commercially desirable fuel cycles and commercially manageable MOX fuel fabrication, testing, qualification, and licensing support activities, are described. The impact of politics and public influences and the necessary role of industry and government contributions are also discussed. (J.P.N.)

Thermal conductivity of heterogeneous LWR MOX fuels

Science.gov (United States)

Staicu, D.; Barker, M.

2013-11-01

It is generally observed that the thermal conductivity of LWR MOX fuel is lower than that of pure UO2. For MOX, the degradation is usually only interpreted as an effect of the substitution of U atoms by Pu. This hypothesis is however in contradiction with the observations of Duriez and Philiponneau showing that the thermal conductivity of MOX is independent of the Pu content in the ranges 3-15 and 15-30 wt.% PuO2 respectively. Attributing this degradation to Pu only implies that stoichiometric heterogeneous MOX can be obtained, while we show that any heterogeneity in the plutonium distribution in the sample introduces a variation in the local stoichiometry which in turn has a strong impact on the thermal conductivity. A model quantifying this effect is obtained and a new set of experimental results for homogeneous and heterogeneous MOX fuels is presented and used to validate the proposed model. In irradiated fuels, this effect is predicted to disappear early during irradiation. The 3, 6 and 10 wt.% Pu samples have a similar thermal conductivity. Comparison of the results for this homogeneous microstructure with MIMAS (heterogeneous) fuel of the same composition showed no difference for the Pu contents of 3, 5.9, 6, 7.87 and 10 wt.%. A small increase of the thermal conductivity was obtained for 15 wt.% Pu. This increase is of about 6% when compared to the average of the values obtained for 3, 6 and 10 wt.% Pu. For comparison purposes, Duriez also measured the thermal conductivity of FBR MOX with 21.4 wt.% Pu with O/M = 1.982 and a density close to 95% TD and found a value in good agreement with the estimation obtained using the formula of Philipponneau [8] for FBR MOX, and significantly lower than his results corresponding to the range 3-15 wt.% Pu. This difference in thermal conductivity is of about 20%, i.e. higher than the measurement uncertainties.Thus, a significant difference was observed between FBR and PWR MOX fuels, but was not explained. This difference

ABB high burnup fuel

International Nuclear Information System (INIS)

Andersson, S.; Helmersson, S.; Nilsson, S.; Jourdain, P.; Karlsson, L.; Limback, M.; Garde, A.M.

1999-01-01

Fuel designed and fabricated by ABB is now operating in 40 PWRs and BWRs in Europe, the United States and Korea. An excellent fuel reliability track record has been established. High burnups are proven for both PWR and BWR. Thermal margin improving features and advanced burnable absorber concepts enable the utilities to adopt demanding duty cycles to meet new economic objectives. In particular we note the excellent reliability record of ABB PWR fuel equipped with Guardian TM debris filter proven to meet the 6 rod-cycles fuel failure goal, and the out-standing operating record of the SVEA 10 x 10 fuel, where ABB is the only vendor to date with batch experience to high burnup. ABB is dedicated to maintain high fuel reliability as well as continually improve and develop a broad line of PWR and BWR products. ABB's development and fuel follow-up activities are performed in close co-operation with its utility customers. This paper provides an overview of recent fuel performance and reliability experience at ABB. Selected development and validation activities for PWR and BWR fuel are presented, for which the ABB test facilities in Windsor (TF-2 loop, mechanical test laboratory) and Vaesteras (FRIGG, BURE) are essential. (authors)

Burnup credit demands for spent fuel management in Ukraine

International Nuclear Information System (INIS)

Medun, V.

2001-01-01

In fact, till now, burnup credit has not be applied in Ukrainian nuclear power for spent fuel management systems (storage and transport). However, application of advanced fuel at VVER reactors, arising spent fuel amounts, represent burnup credit as an important resource to decrease spent fuel management costs. The paper describes spent fuel management status in Ukraine from viewpoint of subcriticality assurance under spent fuel storage and transport. It also considers: 1. Regulation basis concerning subcriticality assurance, 2. Basic spent fuel and transport casks characteristics, 3. Possibilities and demands for burnup credit application at spent fuel management systems in Ukraine. (author)

Development of a fresh MOX fuel transport package for disposition of weapons plutonium

International Nuclear Information System (INIS)

Ludwig, S.B.; Pope, R.B.; Shappert, L.B.; Michelhaugh, R.D.; Chae, S.M.

1998-01-01

The US Department of Energy announced its Record of Decision on January 14, 1997, to embark on a dual-track approach for disposition of surplus weapons-usable plutonium using immobilization in glass or ceramics and burning plutonium as mixed-oxide (MOX) fuel in reactors. In support of the MOX fuel alternative, Oak Ridge National Laboratory initiated development of conceptual designs for a new package for transporting fresh (unirradiated) MOX fuel assemblies between the MOX fabrication facility and existing commercial light-water reactors in the US. This paper summarizes progress made in development of new MOX transport package conceptual designs. The development effort has included documentation of programmatic and technical requirements for the new package and development and analysis of conceptual designs that satisfy these requirements

MTR fuel element burn-up measurements by the reactivity method

International Nuclear Information System (INIS)

Zuniga, A.; Cuya, T.R.; Ravnik, M.

2003-01-01

Fuel element burn-up was measured by the reactivity method in the 10 MW Peruvian MTR reactor RP-10. The main purpose of the experiment was testing the reactivity method for an MTR reactor as the reactivity method was originally developed for TRIGA reactors. The reactivity worth of each measured fuel element was measured in its original core position in order to measure the burn-up of the fuel elements that were part of the experimental core. The burn-up of each measured fuel element was derived by interpolating its reactivity worth from the reactivity worth of two reference fuel elements of known burn-up, whose reactivity worth was measured in the position of the measured fuel element. The accuracy of the method was improved by separating the reactivity effect of burn-up from the effect of the position in the core. The results of the experiment showed that the modified reactivity method for fuel element burn-up determination could be applied also to MTR reactors. (orig.)

Programmatic and technical requirements for the FMDP fresh MOX fuel transport package

International Nuclear Information System (INIS)

Ludwig, S.B.; Michelhaugh, R.D.; Pope, R.B.

1997-12-01

This document is intended to guide the designers of the package to all pertinent regulatory and other design requirements to help ensure the safe and efficient transport of the weapons-grade (WG) fresh MOX fuel under the Fissile Materials Disposition Program. To accomplish the disposition mission using MOX fuel, the unirradiated MOX fuel must be transported from the MOX fabrication facility to one or more commercial reactors. Because the unirradiated fuel contains large quantities of plutonium and is not sufficient radioactive to create a self-protecting barrier to deter the material from theft, DOE intends to use its fleet of safe secure trailers (SSTs) to provide the necessary safeguards and security for the material in transit. In addition to these requirements, transport of radioactive materials must comply with regulations of the Department of Transportation and the Nuclear Regulatory Commission (NRC). In particular, NRC requires that the packages must meet strict performance requirements. The requirements for shipment of MOX fuel (i.e., radioactive fissile materials) specify that the package design is certified by NRC to ensure the materials contained in the packages are not released and remain subcritical after undergoing a series of hypothetical accident condition tests. Packages that pass these tests are certified by NRC as a Type B fissile (BF) package. This document specifies the programmatic and technical design requirements a package must satisfy to transport the fresh MOX fuel assemblies

Fuel analysis code FAIR and its high burnup modelling capabilities

International Nuclear Information System (INIS)

Prasad, P.S.; Dutta, B.K.; Kushwaha, H.S.; Mahajan, S.C.; Kakodkar, A.

1995-01-01

A computer code FAIR has been developed for analysing performance of water cooled reactor fuel pins. It is capable of analysing high burnup fuels. This code has recently been used for analysing ten high burnup fuel rods irradiated at Halden reactor. In the present paper, the code FAIR and its various high burnup models are described. The performance of code FAIR in analysing high burnup fuels and its other applications are highlighted. (author). 21 refs., 12 figs

Advanced fuel cycles and burnup increase of WWER-440 fuel

International Nuclear Information System (INIS)

Proselkov, V.; Saprykin, V.; Scheglov, A.

2003-01-01

Analyses of operational experience of 4.4% enriched fuel in the 5-year fuel cycle at Kola NPP Unit 3 and fuel assemblies with Uranium-Gadolinium fuel at Kola NPP Unit 4 are made. The operability of WWER-440 fuel under high burnup is studied. The obtained results indicate that the fuel rods of WWER-440 assemblies intended for operation within six years of the reviewed fuel cycle totally preserve their operability. Performed analyses have demonstrated the possibility of the fuel rod operability during the fuel cycle. 12 assemblies were loaded into the reactor unit of Kola 3 in 2001. The predicted burnup in six assemblies was 59.2 MWd/kgU. Calculated values of the burnup after operation for working fuel assemblies were ∼57 MWd/kgU, for fuel rods - up to ∼61 MWd/kgU. Data on the coolant activity, specific activity of the benchmark iodine radionuclides of the reactor primary circuit, control of the integrity of fuel rods of the assemblies that were operated for six years indicate that not a single assembly has reached the criterion for the early discharge

Application of reactivity method to MTR fuel burn-up measurement

International Nuclear Information System (INIS)

Zuniga, A.; Ravnik, M.; Cuya, R.

2001-01-01

Fuel element burn-up has been measured for the first time by reactivity method in a MTR reactor. The measurement was performed in RP-10 reactor of Peruvian Institute for Nuclear Energy (IPEN) in Lima. It is a pool type 10MW material testing reactor using standard 20% enriched uranium plate type fuel elements. A fresh element and an element with well defined burn-up were selected as reference elements. Several elements in the core were selected for burn-up measurement. Each of them was replaced in its original position by both reference elements. Change in excess reactivity was measured using control rod calibration curve. The burn-up reactivity worth of fuel elements was plotted as a function of their calculated burnup. Corrected burn-up values of the measured fuel elements were calculated using the fitting function at experimental reactivity for all elements. Good agreement between measured and calculated burn-up values was observed indicating that the reactivity method can be successfully applied also to MTR fuel element burn-up determination.(author)

Novel technique for manipulating MOX fuel particles using radiation pressure of a laser light

International Nuclear Information System (INIS)

Omori, R.

2000-01-01

We have continued theoretical and experimental studies on laser manipulation of nuclear fuel particles, such as UO 2 , PuO 2 and ThO 2 , In this paper, we investigate the applicability of the collection of MOX particles floating in air using radiation pressure of a laser light; some preliminary results are shown. This technique will be useful for removal and confinement of MOX particles being transported by air current or dispersed in a cell box. First, we propose two types of principles for collecting MOX particles. Second, we show some experimental results, Third, we show numerical results of radiation pressure exerted on submicrometer-sized UO 2 particles using Generalized Lorentz-Mie theory. Because optical constants of UO 2 are similar to those of MOX fuel particles, it seems that calculation results obtained hold for MOX fuel particles. 2. Principles of collecting MOX fuel particles using radiation pressure (authors)

Some alternatives to the mixed oxide fuel cycle

International Nuclear Information System (INIS)

Deonigi, D.E.; Eschbach, E.A.; Goldsmith, S.; Pankaskie, P.J.; Rohrmann, C.A.; Widrig, R.D.

1977-02-01

While on initial examination each of the six fuel cycle concepts (tandem cycle, extended burnup, fuel rejuvenation, coprocessing, partial reprocessing, and thorium) described in the report may have some potential for improving safeguards, none of the six appears to have any other major or compelling advantages over the mixed oxide (MOX) fuel cycle. Compared to the MOX cycle, all but coprocessing appear to have major disadvantages, including severe cost penalties. Three of the concepts-tandem, extended burnup, and rejuvenation--share the basic problems of the throwaway cycle (GESMO Alternative 6): without reprocessing, high-level waste volumes and costs are substantially increased, and overall uranium utilization decreases for three reasons. First, the parasitic fission products left in the fuel absorb neutrons in later irradiation steps reducing the overall neutronic efficiencies of these cycles. Second, discarded fuel still has sufficient fissile values to warrant recycle. Third, perhaps most important, the plutonium needed for breeder start-up will not be available; without the breeder, uranium utilization would drop by about a factor of sixty. Two of the concepts--coprocessing and partial reprocessing--involve variations of the basic MOX fuel cycle's chemical reprocessing step to make plutonium diversion potentially more difficult. These concepts could be used with the MOX fuel cycle or in conjunction with the tandem, extended burnup and rejuvenation concepts to eliminate some of the problems with those cycles. But in so doing, the basic impetus for those cycles--elimination of reprocessing for safeguards purposes--no longer exists. Of all the concepts considered, only coprocessing--and particularly the ''master blend'' version--appears to have sufficient promise to warrant a more detailed study. The master blend concept could possibly make plutonium diversion more difficult with minimal impact on the reprocessing and MOX fuel fabrication operations

Safety evaluation on MOX new fuel at marine transport

International Nuclear Information System (INIS)

Tsumune, Daisuke; Ito, Chihiro; Saegusa, Toshiari; Maruyama, Koki

2000-01-01

In the Central Research Institute of Electric Power Industry, in order to confirm effects of MOX new fuel on the public are as small as possible even when its marine transport goes down, some exposed radiation dose has previously conducted on imaginary shipwreck of marine transport on used nuclear fuel, plutonium dioxide, and high level return glass solid. Under a base of such informations, some investigations on safety on marine transport of the MOX new fuel was conducted. On September, 1999, five transport vessels of the MOX new fuel was at first transported on marine. The value of five times of estimated exposed radiation dose (max. 8.1 x 10 -8 mSv/y) corresponds to an evaluation result assumed by shipwreck in marine transport this time. As a result, it was found that the exposed radiation dose estimated on this case would be sufficiently less than an effective dose equivalent limit (1 mSv/y) of public exposure according to the recommendation of ICRP in both coastal and oceanic areas. (G.K.)

Fuel rod behaviour at high burnup WWER fuel cycles

International Nuclear Information System (INIS)

Medvedev, A.; Bogatyr, S.; Kouznetsov, V.; Khvostov, G.; Lagovsky; Korystin, L.; Poudov, V.

2003-01-01

The modernisation of WWER fuel cycles is carried out on the base of complete modelling and experimental justification of fuel rods up to 70 MWd/kgU. The modelling justification of the reliability of fuel rod and fuel rod with gadolinium is carried out with the use of certified START-3 code. START-3 code has a continuous experimental support. The thermophysical and strength reliability of WWER-440 fuel is justified for fuel rod and pellet burnups 65 MWd/kgU and 74 MWd/U, accordingly. Results of analysis are demonstrated by the example of uranium-gadolinium fuel assemblies of second generation under 5-year cycle with a portion of 6-year assemblies and by the example of successfully completed pilot operation of 5-year cycle fuel assemblies during 6 years at unit 3 of Kolskaja NPP. The thermophysical and strength reliability of WWER-1000 fuel is justified for a fuel rod burnup 66 MWd/kgU by the example of fuel operation under 4-year cycles and 6-year test operation of fuel assemblies at unit 1 of Kalininskaya NPP. By the example of 5-year cycle at Dukovany NPP Unit 2 it was demonstrated that WWER fuel rod of a burnup 58 MWd/kgU ensure reliable operation under load following conditions. The analysis has confirmed sufficient reserves of Russian fuel to implement program of JSC 'TVEL' in order to improve technical and economical parameters of WWER fuel cycles

Thorium utilization in a small long-life HTR. Part I: Th/U MOX fuel blocks

Energy Technology Data Exchange (ETDEWEB)

Ding, Ming, E-mail: dingm2005@gmail.com [Delft University of Technology, Reactor Institute Delft, Mekelweg 15, 2629 JB, Delft (Netherlands); Harbin Engineering University, Nantong Street 145, 150001 Harbin (China); Kloosterman, Jan Leen, E-mail: j.l.kloosterman@tudelft.nl [Delft University of Technology, Reactor Institute Delft, Mekelweg 15, 2629 JB, Delft (Netherlands)

2014-02-15

Highlights: • We propose thorium MOX (TMOX) fuel blocks for a small block-type HTR. • The TMOX fuel blocks with low-enriched uranium are recommended. • More thorium decreases the reactivity swing of the TMOX fuel blocks. • Thorium reduces the negative temperature coefficient of the TMOX fuel blocks. • Thorium increases the conversion ratio of the TMOX fuel blocks. - Abstract: The U-Battery is a small, long-life and transportable high temperature gas-cooled reactor (HTR). The neutronic features of a typical fuel block with uranium and thorium have been investigated for a application of the U-Battery, by parametrically analyzing the composition and geometric parameters. The type of fuel block is defined as Th/U MOX fuel block because uranium and thorium are assumed to be mixed in each fuel kernel as a form of (Th,U)O{sub 2}. If the initially loaded mass of U-235 is mostly consumed in the early period of the lifetime of Th/U MOX fuel block, low-enriched uranium (LEU) as ignited fuel will not largely reduce the neutronic performance of the Th/U MOX fuel block, compared with high-enriched uranium. The radii of fuel kernels and fuel compacts and packing fraction of TRISO particles determine the atomic ratio of the carbon to heavy metal. When the ratio is smaller than 400, the difference among them due to double heterogeneous effects can be neglected for the Th/U MOX fuel block. In the range between 200 and 400, the reactivity swing of the Th/U MOX fuel block during 10 years is sufficiently small. The magnitude of the negative reactivity temperature coefficients of the Th/U MOX fuel block decreases by 20–45%, which is positive to reduce temperature defect of the Th/U MOX fuel block. The conversion ratio (CR) of the fuel increases from 0.48 (typical CR of the LEU-fueled U-Battery) to 0.78. The larger conversion ratio of the Th/U MOX fuel block reduces the reactivity swing during 10 years for the U-Battery.

A model for the description of the evolution of PU agglomerates in MOX fuels

Energy Technology Data Exchange (ETDEWEB)

Federici, E [CEA Centre d` Etudes de Cadarache, 13 - Saint-Paul-lez-Durance (France); Blanpain, P [FRAMATOME, Lyon (France); Permezel, P [Electricite de France, Moret-sur-Loing (France)

1997-08-01

In order to describe the irradiation behavior of Pu agglomerates under LWR steady state conditions in MIMAS MOX fuels, a model including the neutronic evolution of the heavy atoms and their diffusion processes between the agglomerates and the matrix has been developed. It leads to the calculations of Pu enrichment in the two phases and of the agglomerates size evolution during irradiation. The calculated distribution of the fission in the fuel gives access to the local power and burnup heterogeneity factor. Electron probe microanalyses (EPMA) have been carried out on fuels irradiated up to 45000 MWd/tM. Diametral and local distribution of Pu are used to calculate the enrichments of the agglomerates and the matrix, which are then compared to the results of the model. During irradiation, the Pu concentration falls markedly in the agglomerates and increases steadily in the matrix, leading to a homogenization of the fuel on a microstructural scale. Heterogeneity factors give an estimate of the deviation from homogeneity. Knowing the local fission rate and burnup in the agglomerates and the matrix enables the calculation of the local fission gas concentrations, which are compared to the xenon EPMA diametral distribution. Comparison with the calculated matrix xenon concentration at the edge of the pellet where there is no gas release, shows that some fission gas atoms which originated from the agglomerates, have been dissolved in the matrix by recoil. The calculated gas concentrations give an estimate of the quantity of gas dissolved. This work has been performed with the intent to improved fuel rod performance code estimates of fission gas concentrations retained or released in both the matrix and the agglomerates. (author). 4 refs, 7 figs.

A model for the description of the evolution of PU agglomerates in MOX fuels

International Nuclear Information System (INIS)

Federici, E.; Blanpain, P.; Permezel, P.

1997-01-01

In order to describe the irradiation behavior of Pu agglomerates under LWR steady state conditions in MIMAS MOX fuels, a model including the neutronic evolution of the heavy atoms and their diffusion processes between the agglomerates and the matrix has been developed. It leads to the calculations of Pu enrichment in the two phases and of the agglomerates size evolution during irradiation. The calculated distribution of the fission in the fuel gives access to the local power and burnup heterogeneity factor. Electron probe microanalyses (EPMA) have been carried out on fuels irradiated up to 45000 MWd/tM. Diametral and local distribution of Pu are used to calculate the enrichments of the agglomerates and the matrix, which are then compared to the results of the model. During irradiation, the Pu concentration falls markedly in the agglomerates and increases steadily in the matrix, leading to a homogenization of the fuel on a microstructural scale. Heterogeneity factors give an estimate of the deviation from homogeneity. Knowing the local fission rate and burnup in the agglomerates and the matrix enables the calculation of the local fission gas concentrations, which are compared to the xenon EPMA diametral distribution. Comparison with the calculated matrix xenon concentration at the edge of the pellet where there is no gas release, shows that some fission gas atoms which originated from the agglomerates, have been dissolved in the matrix by recoil. The calculated gas concentrations give an estimate of the quantity of gas dissolved. This work has been performed with the intent to improved fuel rod performance code estimates of fission gas concentrations retained or released in both the matrix and the agglomerates. (author). 4 refs, 7 figs

Development and verification of Monte Carlo burnup calculation system

International Nuclear Information System (INIS)

Ando, Yoshihira; Yoshioka, Kenichi; Mitsuhashi, Ishi; Sakurada, Koichi; Sakurai, Shungo

2003-01-01

Monte Carlo burnup calculation code system has been developed to evaluate accurate various quantities required in the backend field. From the Actinide Research in a Nuclear Element (ARIANE) program, by using, the measured nuclide compositions of fuel rods in the fuel assemblies irradiated in the commercial Netherlands BWR, the analyses have been performed for the code system verification. The code system developed in this paper has been verified through analysis for MOX and UO2 fuel rods. This system enables to reduce large margin assumed in the present criticality analysis for LWR spent fuels. (J.P.N.)

Characterization of candidate DOE sites for fabricating MOX fuel for lead assemblies

Energy Technology Data Exchange (ETDEWEB)

Holdaway, R.F.; Miller, J.W.; Sease, J.D.; Moses, R.J.; O`Connor, D.G. [Oak Ridge National Lab., TN (United States); Carrell, R.D. [Technical Resources International, Inc., Richland, WA (United States); Jaeger, C.D. [Sandia National Labs., Albuquerque, NM (United States); Thompson, M.L.; Strasser, A.A. [Delta-21 Resources, Inc., Oak Ridge, TN (United States)

1998-03-01

The Office of Fissile Materials Disposition (MD) of the Department of Energy (DOE) is directing the program to disposition US surplus weapons-usable plutonium. For the reactor option for disposition of this surplus plutonium, MD is seeking to contract with a consortium, which would include a mixed-oxide (MOX) fuel fabricator and a commercial US reactor operator, to fabricate and burn MOX fuel in existing commercial nuclear reactors. This option would entail establishing a MOX fuel fabrication facility under the direction of the consortium on an existing DOE site. Because of the lead time required to establish a MOX fuel fabrication facility and the need to qualify the MOX fuel for use in a commercial reactor, MD is considering the early fabrication of lead assemblies (LAs) in existing DOE facilities under the technical direction of the consortium. The LA facility would be expected to produce a minimum of 1 metric ton heavy metal per year and must be operational by June 2003. DOE operations offices were asked to identify candidate sites and facilities to be evaluated for suitability to fabricate MOX fuel LAs. Savannah River Site, Argonne National Laboratory-West, Hanford, Lawrence Livermore National Laboratory, and Los Alamos National Laboratory were identified as final candidates to host the LA project. A Site Evaluation Team (SET) worked with each site to develop viable plans for the LA project. SET then characterized the suitability of each of the five plans for fabricating MOX LAs using 28 attributes and documented the characterization to aid DOE and the consortium in selecting the site for the LA project. SET concluded that each option has relative advantages and disadvantages in comparison with other options; however, each could meet the requirements of the LA project as outlined by MD and SET.

Characterization of candidate DOE sites for fabricating MOX fuel for lead assemblies

International Nuclear Information System (INIS)

Holdaway, R.F.; Miller, J.W.; Sease, J.D.; Moses, R.J.; O'Connor, D.G.; Carrell, R.D.; Jaeger, C.D.; Thompson, M.L.; Strasser, A.A.

1998-03-01

The Office of Fissile Materials Disposition (MD) of the Department of Energy (DOE) is directing the program to disposition US surplus weapons-usable plutonium. For the reactor option for disposition of this surplus plutonium, MD is seeking to contract with a consortium, which would include a mixed-oxide (MOX) fuel fabricator and a commercial US reactor operator, to fabricate and burn MOX fuel in existing commercial nuclear reactors. This option would entail establishing a MOX fuel fabrication facility under the direction of the consortium on an existing DOE site. Because of the lead time required to establish a MOX fuel fabrication facility and the need to qualify the MOX fuel for use in a commercial reactor, MD is considering the early fabrication of lead assemblies (LAs) in existing DOE facilities under the technical direction of the consortium. The LA facility would be expected to produce a minimum of 1 metric ton heavy metal per year and must be operational by June 2003. DOE operations offices were asked to identify candidate sites and facilities to be evaluated for suitability to fabricate MOX fuel LAs. Savannah River Site, Argonne National Laboratory-West, Hanford, Lawrence Livermore National Laboratory, and Los Alamos National Laboratory were identified as final candidates to host the LA project. A Site Evaluation Team (SET) worked with each site to develop viable plans for the LA project. SET then characterized the suitability of each of the five plans for fabricating MOX LAs using 28 attributes and documented the characterization to aid DOE and the consortium in selecting the site for the LA project. SET concluded that each option has relative advantages and disadvantages in comparison with other options; however, each could meet the requirements of the LA project as outlined by MD and SET

Experiences with the first prototype MOX fuel rods fabricated at Argentina

International Nuclear Information System (INIS)

Marino, Armando Carlos; Perez, Edmundo; Adelfang, Pablo

1996-01-01

The irradiation of the first Argentine prototypes of pressurized heavy water reactor (PHWR) (U,Pu)O sub 2 MOX fuels began in 1986. These experiments were carried out in the High Flux Reactor (HFR)-Petten, Holland. The rods were prepared and controlled in the C NEA's alpha Facility. The first rod has been used for destructive pre-irradiation analysis. The second one as a pathfinder to adjust systems in the HFR. Two additional rods including iodine doped pellets were intended to simulate 15000 MWd/T(M) burnup. The remaining two rods were irradiated until 15000 MWd/T(M). One of them underwent a final ramp with the aim of verifying fabrication processes and studying the behaviour under power transients. BACO (BArra COmbustible) code was used to define the power histories and to analyse the experiments. This paper presents a description of the different experiments and a comparison between the results of the postirradiation examinations and the BACO outputs

From Russian weapons grade plutonium to MOX fuel

International Nuclear Information System (INIS)

Braehler, G.; Kudriavtsev, E.G.; Seyve, C.

1997-01-01

The April 1996, G7 Moscow Summit on nuclear matters provided a political framework for one of the most current significant challenges: ensuring a consistent answer to the weapons grade fissile material disposition issue resulting from the disarmament effort engaged by both the USA and Russia. International technical assessments have showed that the transformation of Weapons grade Plutonium in MOX fuel is a very efficient, safe, non proliferant and economically effective solution. In this regard, COGEMA and SIEMENS, have set up a consistent technical program properly addressing incineration of weapons grade plutonium in MOX fuels. The leading point of this program would be the construction of a Weapons grade Plutonium dedicated MOX fabrication plant in Russia. Such a plant would be based on the COGEMA-SIEMENS industrial capabilities and experience. This facility would be operated by MINATOM which is the partner for COGEMA-SIEMENS. MINATOM is in charge of coordination of the activity of the Russian research and construction institutes. The project take in account international standards for non-proliferation, safety and waste management. France and Germany officials reasserted this position during their last bilateral summits held in Fribourg in February and in Dijon in June 1996. MINATOM and the whole Russian nuclear community have already expressed their interest to cooperate with COGEMA-SIEMENS in the MOX field. This follows governmental-level agreements signed in 1992 by French, German and Russian officials. For years, Russia has been dealing with research and development on MOX fabrication and utilization. So, the COGEMA-SIEMENS MOX proposal gives a realistic answer to the management of weapons grade plutonium with regard to the technical, industrial, cost and schedule factors. (author)

Study of the lattice parameter evolution of PWR irradiated MOX fuel by X-Ray diffraction

International Nuclear Information System (INIS)

Clavier, B.

1995-01-01

Fuel irradiation leads to a swelling resulting from the formation of gaseous (Kr, Xe) or solid fission products which are found either in solution or as solid inclusions in the matrix. This phenomena has to be evaluated to be taken into account in fuel cladding Interaction. Fuel swelling was studied as a function of burn up by measuring the corresponding cell constant evolution by X-Ray diffraction. This study was realized on Mixed Oxide Fuels (MOX) irradiated in a Pressurized Water Reactor (PWR) at different burn-up for 3 initial Pu contents. Lattice parameter evolutions were followed as a function of burn-up for the irradiated fuel with and without an annealing thermal treatment. These experimental evolutions are compared to the theoretical evolutions calculated from the hard sphere model, using the fission product concentrations determined by the APPOLO computer code. Contribution of varying parameters influencing the unit cell value is discussed. Thermal treatment effects were checked by metallography, X-Ray diffraction and microprobe analysis. After thermal treatment, no structural change was observed but a decrease of the lattice parameter was measured. This modification results essentially from self-irradiation defect annealing and not from stoichiometry variations. Microprobe analysis showed that about 15% of the formed Molybdenum is in solid solution In the oxide matrix. Micrographs showed the existence of Pu packs in the oxide matrix which induces a broadening of diffraction lines. The RIETVELD method used to analyze the X-Ray patterns did not allow to characterize independently the Pu packs and the oxide matrix lattice parameters. Nevertheless, with this method, the presence of micro-strains in the irradiated nuclear fuel could be confirmed. (author)

ORIGEN2 libraries based on JENDL-3.2 for LWR-MOX fuels

Energy Technology Data Exchange (ETDEWEB)

Suyama, Kenya; Katakura, Jun-ichi [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment; Onoue, Masaaki; Matsumoto, Hideki [Mitsubishi Heavy Industries Ltd., Tokyo (Japan); Sasahara, Akihiro [Central Research Inst. of Electric Power Industry, Tokyo (Japan)

2000-11-01

A set of ORIGEN2 libraries for LWR MOX fuels was developed based on JENDL-3.2. The libraries were compiled with SWAT using the specification of MOX fuels that will be used in nuclear power reactors in Japan. The verification of the libraries were performed by the analyses of post irradiation examinations for the fuels from European PWR. By the analysis of PIE data from PWR in United States, the comparison was made between calculation and experimental results in the case of that parameters for making the libraries are different from irradiation conditions. These new libraries for LWR MOX fuels are packaged in ORLIBJ32, the libraries released in 1999. (author)

Fuel production for LWRs - MOX fuel aspects

International Nuclear Information System (INIS)

Deramaix, P.

2005-01-01

Plutonium recycling in Light Water Reactors is today an industrial reality. It is recycled in the form of (U, Pu)O 2 fuel pellets (MOX), fabricated to a large extent according to UO 2 technology and pellet design. The similarity of physical, chemical, and neutron properties of both fuels also allows MOX fuel to be burnt in nuclear plants originally designed to burn UO 2 . The industrial processes presently in use or planned are all based on a mechanical blending of UO 2 and PuO 2 powders. To obtain finely dispersed plutonium and to prevent high local concentration of plutonium, the feed materials are micronised. In the BNFL process, the whole (UO 2 , PuO 2 ) blend is micronised by attrition milling. According to the MIMAS process, developed by BELGONUCLEAIRE, a primary blend made of UO 2 containing about 30% PuO 2 is micronised in a ball mill, afterwards this primary blend is mechanically diluted in UO 2 to obtain the specified Pu content. After mixing, the (U, Pu)O 2 powder is pressed and the pellets are sintered. The sintering cover gas contains moisture and 5 v/o H 2 . Moisture increases the sintering process and the U-Pu interdiffusion. After sintering and grinding, the pellets are submitted to severe controls to verify conformity with customer specifications (fissile content, Pu distribution, surface condition, chemical purity, density, microstructure). (author)

A fission gas release model for MOX fuel and its verification

International Nuclear Information System (INIS)

Koo, Y.H.; Sohn, D.S.; Strijov, P.

2000-01-01

A fission gas release model for MOX fuel has been developed based on a model for UO 2 fuel. Using the concept of equivalent cell, the model considers the uneven distribution of Pu within the fuel matrix and a number of Pu-rich particles that could lead to a non-uniform fission rate and fission gas distribution across the fuel pellet. The model has been incorporated into a code, COSMOS, and some parametric studies were made to analyze the effect of the size and Pu content of Pu-rich agglomerates. The model was then applied to the experimental data obtained from the FIGARO program, which consisted of the base irradiation of MOX fuels in the BEZNAU-1 PWR and the subsequent irradiation of four refabricated fuel segments in the Halden reactor. The calculated gas releases show good agreement with the measured ones. In addition, the present analysis indicates that the microstructure of the MOX fuel used in the FIGARO program is such that it has produced little difference in terms of gas release compared with UO 2 fuel. (author)

Benchmark calculations for VENUS-2 MOX -fueled reactor dosimetry

International Nuclear Information System (INIS)

Kim, Jong Kung; Kim, Hong Chul; Shin, Chang Ho; Han, Chi Young; Na, Byung Chan

2004-01-01

As a part of a Nuclear Energy Agency (NEA) Project, it was pursued the benchmark for dosimetry calculation of the VENUS-2 MOX-fueled reactor. In this benchmark, the goal is to test the current state-of-the-art computational methods of calculating neutron flux to reactor components against the measured data of the VENUS-2 MOX-fuelled critical experiments. The measured data to be used for this benchmark are the equivalent fission fluxes which are the reaction rates divided by the U 235 fission spectrum averaged cross-section of the corresponding dosimeter. The present benchmark is, therefore, defined to calculate reaction rates and corresponding equivalent fission fluxes measured on the core-mid plane at specific positions outside the core of the VENUS-2 MOX-fuelled reactor. This is a follow-up exercise to the previously completed UO 2 -fuelled VENUS-1 two-dimensional and VENUS-3 three-dimensional exercises. The use of MOX fuel in LWRs presents different neutron characteristics and this is the main interest of the current benchmark compared to the previous ones

The development of B.N.F.L.'S MOX fuel supply business

International Nuclear Information System (INIS)

Edwards, J.; Brown, C.; Marshall, S.J.; Connell, M.; Thompson, H.

1998-01-01

In 1990 BNFL developed a strategy to become one of the world leading MOX fuel suppliers. This strategy involved the design, construction and operation of a small scale demonstration plant known as the MOX Demonstration Facility (MDF) and a large scale facility known as the Sellafield MOX Plant (SMP). To support the development of these facilities, BNFL developed a new MOX fuel fabrication process known as the Short Binderless Route (SBR). Since the 1990 decision was made, the company has successfully built, commissioned and operated the MDF, and has designed, built and is in the process of commissioning the 120 t(HM)/year SMP. The scale of the business has thus developed significantly and the direction and prospects for the future of the business are clear and well understood, with the focus being on the use of BNFL technology to produce quality MOX fuel to meet customers' requirements. This paper reviews the development of BNFL's MOX business and describes the technology being used in the state of the art SMP. The paper also explains the approach taken to commission the plant and how key safety features have been incorporated into the design. Up to date information on the performance of Short Binderless Route fuel is provided, and the future development of the business is discussed. (author)

RIA tests in CABRI with MOX fuel

International Nuclear Information System (INIS)

Schmitz, F.; Papin, J.; Gonnier, C.

2000-01-01

Three MOX-fuel tests have been successfully performed within the framework of the CABRI REP-Na test program. From the experimental findings which are presently available, no evidence for thermal effects resulting from the heterogeneous nature of the fuel can be given. There are very clear hints however that fission gas effects are enhanced with regard to the behaviour of UO 2 . The clad rupture observed in REP-Na 7 is of different nature than the failures observed in Cabri tests with UO 2 fuel. Failures of UO 2 fuel rods only occurred when the clad mechanical properties were severely affected by the presence of hydride blisters, while in REP-Na 7 a clear indication is made that the loading potential of the MOX fuel pellets was high enough to break a sound cladding. Concerning the transient fuel behaviour after reaching the critical heat-flux under reactor typical conditions (pressure, temperature and flow), no data base could be provided by the tests in the present sodium test loop (as for the UO 2 fuel behaviour). The IPSN project to implement into the Cabri reactor a pressurised water loop which will allow to simulate the complete RIA accident sequence under PWR reactor typical conditions, aims at providing this missing data base. (author)

LWR mox fuel experience in Belgium and France with special emphasis on results obtained in BR3

International Nuclear Information System (INIS)

Bairiot, H.; Haas, D.; Lippens, M.; Motte, F.; Lebastard, G.; Marin, J.F.

1986-09-01

The course of the paper reflects two main topics: LWR MOX fuel experience in Belgium and France, summarizing the fabrication techniques, the references, the underlying MOX fuel technology and the current R and D programs for expanding the data base; behaviour of MOX fuel rods irradiated under steady state and transient operating conditions, focusing on MOX fuel technology features acquired through the irradiations performed in the BR3 PWR, supplemented by tests in the BR2 MTR. This paper focuses on the thermomechanical behaviour of LWR MOX fuel rods, which is intimately related to the fabrication technique and vice-versa. 22 refs

Validation of the Nuclear Design Method for MOX Fuel Loaded LWR Cores

International Nuclear Information System (INIS)

Saji, E.; Inoue, Y.; Mori, M.; Ushio, T.

2001-01-01

The actual batch loading of mixed-oxide (MOX) fuel in light water reactors (LWRs) is now ready to start in Japan. One of the efforts that have been devoted to realizing this batch loading has been validation of the nuclear design methods calculating the MOX-fuel-loaded LWR core characteristics. This paper summarizes the validation work for the applicability of the CASMO-4/SIMULATE-3 in-core fuel management code system to MOX-fuel-loaded LWR cores. This code system is widely used by a number of electric power companies for the core management of their commercial LWRs. The validation work was performed for both boiling water reactor (BWR) and pressurized water reactor (PWR) applications. Each validation consists of two parts: analyses of critical experiments and core tracking calculations of operating plants. For the critical experiments, we have chosen a series of experiments known as the VENUS International Program (VIP), which was performed at the SCK/CEN MOL laboratory in Belgium. VIP consists of both BWR and PWR fuel assembly configurations. As for the core tracking calculations, the operating data of MOX-fuel-loaded BWR and PWR cores in Europe have been utilized

Fuel burnup analysis for the Moroccan TRIGA research reactor

International Nuclear Information System (INIS)

El Bakkari, B.; El Bardouni, T.; Nacir, B.; El Younoussi, C.; Boulaich, Y.; Boukhal, H.; Zoubair, M.

2013-01-01

Highlights: ► A fuel burnup analysis of the 2 MW TRIGA MARK II Moroccan research reactor was established. ► Burnup calculations were done by means of the in-house developed burnup code BUCAL1. ► BUCAL1 uses the MCNP tallies directly in the calculation of the isotopic inventories. ► The reactor life time was found to be 3360 MW h considering full power operating conditions. ► Power factors and fluxes of the in-core irradiation positions are strongly affected by burnup. -- Abstract: The fundamental advantage and main reason to use Monte Carlo methods for burnup calculations is the possibility to generate extremely accurate burnup dependent one group cross-sections and neutron fluxes for arbitrary core and fuel geometries. Yet, a set of values determined for a material at a given position and time remains accurate only in a local region, in which neutron spectrum and flux vary weakly — and only for a limited period of time, during which changes of the local isotopic composition are minor. This paper presents the approach of fuel burnup evaluation used at the Moroccan TRIGA MARK II research reactor. The approach is essentially based upon the utilization of BUCAL1, an in-house developed burnup code. BUCAL1 is a FORTRAN computer code designed to aid in analysis, prediction, and optimization of fuel burnup performance in nuclear reactors. The code was developed to incorporate the neutron absorption reaction tally information generated directly by MCNP5 code in the calculation of fissioned or neutron-transmuted isotopes for multi-fueled regions. The fuel cycle length and changes in several core parameters such as: core excess reactivity, control rods position, fluxes at the irradiation positions, axial and radial power factors and other parameters are estimated. Besides, this study gives valuable insight into the behavior of the reactor and will ensure better utilization and operation of the reactor during its life-time and it will allow the establishment of

Preliminary analysis of a large 1600 MWe PWR core loaded with 30% MOX fuel

International Nuclear Information System (INIS)

Polidoro, Franco; Corsetti, Edoardo; Vimercati, Giuliano

2011-01-01

The paper presents a full-core 3-D analysis of the performances of a large 1600 MWe PWR core, loaded with 30% MOX fuel, in accordance with the European Utility Requirements (EUR). These requirements state that the European next generation power plants have to be designed capable to use MOX (UO 2 - PuO 2 ) fuel assemblies up to 50% of the core, together with UO 2 fuel assemblies. The use of MOX assemblies has a significant impact on key physic parameters and on safety. A lot of studies have been carried out in the past to explore the feasibility of plutonium recycling strategies by loading LWR reactors with MOX fuel. Many of these works were based on lattice codes, in order to perform detailed analyses of the neutronic characteristics of MOX assemblies. With the aim to take into account their interaction with surrounding UO 2 fuel elements, and the global effects on the core at operational conditions, an integrated approach making use of a 3-D core simulation is required. In this light, the present study adopts the state-of-art numerical models CASMO-5 and SIMULATE-3 to analyze the behavior of the core fueled with 30% MOX and to compare it with that of a large PWR reference core, fueled with UO 2 . (author)

Estimate of the instant release fraction for UO2 and MOX fuel at t=0

International Nuclear Information System (INIS)

Johnson, L.; Poinssot, C; Ferry, C.; Lovera, P.

2004-07-01

values, which results in significant overprediction of average IRF values. Best estimate IRF values are determined for moderate burnup UO 2 fuel for nuclides for which data exist, because the understanding and data is sufficient. Only pessimistic IRF values are estimated for radionuclides for which little data is available and in the case of MOX fuel and higher burnup UO 2 fuel. Special attention is given to several phenomena occurring in the outer region of fuel pellets (rim region) resulting in restructuring of fuel grains. These include: a) high fission density as a result of high yields of 239 Pu arising from capture of epithermal neutrons; b) increased porosity; c) reduction in grain size; d) increased thermal release of fission gas from the grains. From the perspective of assessing the release of fission products from spent fuel under disposal conditions, the restructuring process is important

Analysis of high burnup pressurized water reactor fuel using uranium, plutonium, neodymium, and cesium isotope correlations with burnup

International Nuclear Information System (INIS)

Kim, Jung Suk; Jeon, Young Shin; Park, Soon Dal; Ha, Yeong Keong; Song, Kyu Seok

2015-01-01

The correlation of the isotopic composition of uranium, plutonium, neodymium, and cesium with the burnup for high burnup pressurized water reactor fuels irradiated in nuclear power reactors has been experimentally investigated. The total burnup was determined by Nd-148 and the fractional 235 U burnup was determined by U and Pu mass spectrometric methods. The isotopic compositions of U, Pu, Nd, and Cs after their separation from the irradiated fuel samples were measured using thermal ionization mass spectrometry. The contents of these elements in the irradiated fuel were determined through an isotope dilution mass spectrometric method using 233 U, 242 Pu, 150 Nd, and 133 Cs as spikes. The activity ratios of Cs isotopes in the fuel samples were determined using gamma-ray spectrometry. The content of each element and its isotopic compositions in the irradiated fuel were expressed by their correlation with the total and fractional burnup, burnup parameters, and the isotopic compositions of different elements. The results obtained from the experimental methods were compared with those calculated using the ORIGEN-S code

Fuel R and D international programmes, a way to demonstrate future fuel performances

International Nuclear Information System (INIS)

Vanderborck, Y.; Mertens, L.; Dekeyser, J.; Sannen, L.

1997-01-01

As a MOX fuel manufacturer, BELGONUCLEAIRE have spent more than 15 years promoting and managing International R and D Programmes, many of them in close cooperation with SCK''centrdot'' CEN. Such programmes dedicated to MOX versus UO 2 fuel behaviour are most of the time based on irradiation in research reactors in which the investigated fuel is submitted to power variations and to ramp testing or are performed in commercial reactors. This paper is focused on recent programmes concerned by high and medium burn-up in BWR and PWR conditions for MOX fuel. It will present also the new opportunities for new programmes. The goals, the programmes descriptions and the expected data being part of these R and D programmes is presented. (author)

Burnup determination of mass spectrometry for nuclear fuels

International Nuclear Information System (INIS)

Zhang Chunhua.

1987-01-01

The various methods currently being used in burnup determination of nuclear fuels are studied and reviewed. The mass spectrometry method of destructive testing is discussed emphatically. The burnup determination of mass spectrometry includes heavy isotopic abundance ratio method and isotope dilution mass spectrometry used as burnup indicator for the fission products. The former is applied to high burnup level, but the later to various burnup level. According to experiences, some problems which should be noticed in burnup determination of mass spectrometry are presented

Irradiation of Argentine MOX fuels: Post-irradiation results and analysis

International Nuclear Information System (INIS)

Marino, A.C.; Perez, E.; Adelfang, P.

1997-01-01

The irradiation of the first Argentine prototypes of PHWR MOX fuels began in 1986. These experiments were made in the HFR-Petten reactor, Holland. The rods were prepared and controlled in the CNEA's facility. The postirradiation examinations were performed in the Kernforschungszentrum, Karlsruhe, Germany and in the JRC, Petten. The first rod has been used for destructive pre-irradiation analysis. The second one as a pathfinder to adjust systems in the HFR. Two additional rods including iodine doped pellets were intended to simulate 15000 MWd/T(M) burnup. The remaining two rods were irradiated until 15000 MWd/T(M) (BU15 experiment). One of them underwent a final ramp with the aim of verifying fabrication processes and studying the behaviour under power transients. BACO code was used to define the power histories and to analyze the experiments. This paper presents the postirradiation examinations for the BU15 experiments and a comparison with the BACO outputs for the rod that presented a failure during the ramp test of the BU15 experiment. (author). 17 refs, 30 figs, 5 tabs

Implement of MOX fuel assemblies in the design of the fuel reload for a BWR; Implemento de ensambles de combustible MOX en el diseno de la recarga de combustible para un BWR

Energy Technology Data Exchange (ETDEWEB)

Enriquez C, P.; Ramirez S, J. R.; Alonso V, G.; Palacios H, J. C., E-mail: pastor.enriquez@inin.gob.mx [ININ, Carretera Mexico-Toluca s/n, 52750 Ocoyoacac, Estado de Mexico (Mexico)

2011-11-15

At the present time the use of mixed oxides as nuclear fuel is a technology that has been implemented in mixed reloads of fuel for light water reactors. Due to the plutonium production in power reactors, is necessary to realize a study that presents the plutonium use like nuclear fuel. In this work a study is presented that has been carried out on the design of a fuel assembly with MOX to be proposed in the supply of a fuel reload. The fissile relationship of uranium to plutonium is presented for the design of the MOX assembly starting from plutonium recovered in the reprocessing of spent fuel and the comparison of the behavior of the infinite multiplication factor is presented and of the local power peak factor, parameters of great importance in the fuel assemblies design. The study object is a fuel assembly 10 x 10 GNF2 type for a boiling water reactor. The design of the fuel reload pattern giving fuel assemblies with MOX, so the comparison of the behavior of the stop margin for a fuel reload with UO{sub 2} and a mixed reload, implementing 12 and 16 fuel assemblies with MOX are presented. The results show that the implement of fuel assemblies with MOX in a BWR is possible, but this type of fuels creates new problems that are necessary to study with more detail. In the development of this work the calculus tools were the codes: INTREPIN-3, CASMO-4, CMSLINK and SIMULATE-3. (Author)

International symposium on MOX fuel cycle technologies for medium and long-term deployment. Book of extended synopses

International Nuclear Information System (INIS)

1999-05-01

The purpose of the Symposium was to provide a forum to exchange information on MOX fuel cycle technologies with focus on how past experience is being or can be used to progress further, either for facing more demanding fabrication and utilization conditions or for extending into new processing or utilization domains. Presented papers covered the following topics: Current status and prospects concerning plutonium management and MOX fuel utilization; MOX fuel fabrication technology and quality control; Fuel design, performance and testing; In-core fuel management and advanced fuel cycle options; Safety analysis, licensing and safeguards; Transportation and management of irradiated MOX fuel

Investigation on spent fuel characteristics of reduced-moderation water reactor (RMWR)

International Nuclear Information System (INIS)

Fukaya, Y.; Okubo, T.; Uchikawa, S.

2008-01-01

The spent fuel characteristics of the reduced-moderation water reactor (RMWR) have been investigated using the SWAT and ORIGEN codes. RMWR is an advanced LWR concept for plutonium recycling by using the MOX fuel. In the code calculation, the ORIGEN libraries such as one-group cross-section data prepared for RMWR were necessary. Since there were no open libraries for RMWR, they were produced in this study by using the SWAT code. New libraries based on the heterogeneous core modeling in the axial direction and with the variable actinide cross-section (VXSEC) option were produced and selected as the representative ORIGEN libraries for RMWR. In order to investigate the characteristics of the RMWR spent fuel, the decay heat, the radioactivity and the content of each nuclide were evaluated with ORIGEN using these libraries. In this study, the spent fuel characteristics of other types of reactors, such as PWR, BWR, high burn-up PWR, full-MOX-PWR, full-MOX-BWR and FBR, were also evaluated with ORIGEN. It has been found that about a half of the decay heat of the RMWR spent fuel comes from the actinides nuclides. It is the same with the radioactivity. The decay heat and the radioactivity of the RMWR spent fuel are lower than those of full-MOX-LWRs and FBR, and are the same level as those of the high burn-up PWR. The decay heat and the radioactivity from the fission products (FPs) in the spent fuel mainly depend on the burn-up and the burn-up time rather than the reactor type. Therefore, the decay heat and the radioactivity from FPs in the RMWR spent fuel are smaller, reflecting its relatively long burn-up time resulted from its core characteristics with the high conversion ratio. The radioactivity from the actinides in the spent fuel mainly depends on the 241 Pu content in the initial fuel, and the decay heat mainly depends on 238 Pu and 244 Cm. The contribution of 244 Cm is much smaller in RMWR than in MOX-LWRs because of the difference in the spectrum. In addition, from

Investigation on spent fuel characteristics of reduced-moderation water reactor (RMWR)

Energy Technology Data Exchange (ETDEWEB)

Fukaya, Y. [Advanced Nuclear System Research and Development Directorate, Japan Atomic Energy Agency (JAEA), Oarai-machi, Ibaraki-ken 311-1393 (Japan)], E-mail: fukaya.yuji@jaea.go.jp; Okubo, T.; Uchikawa, S. [Advanced Nuclear System Research and Development Directorate, Japan Atomic Energy Agency (JAEA), Oarai-machi, Ibaraki-ken 311-1393 (Japan)

2008-07-15

The spent fuel characteristics of the reduced-moderation water reactor (RMWR) have been investigated using the SWAT and ORIGEN codes. RMWR is an advanced LWR concept for plutonium recycling by using the MOX fuel. In the code calculation, the ORIGEN libraries such as one-group cross-section data prepared for RMWR were necessary. Since there were no open libraries for RMWR, they were produced in this study by using the SWAT code. New libraries based on the heterogeneous core modeling in the axial direction and with the variable actinide cross-section (VXSEC) option were produced and selected as the representative ORIGEN libraries for RMWR. In order to investigate the characteristics of the RMWR spent fuel, the decay heat, the radioactivity and the content of each nuclide were evaluated with ORIGEN using these libraries. In this study, the spent fuel characteristics of other types of reactors, such as PWR, BWR, high burn-up PWR, full-MOX-PWR, full-MOX-BWR and FBR, were also evaluated with ORIGEN. It has been found that about a half of the decay heat of the RMWR spent fuel comes from the actinides nuclides. It is the same with the radioactivity. The decay heat and the radioactivity of the RMWR spent fuel are lower than those of full-MOX-LWRs and FBR, and are the same level as those of the high burn-up PWR. The decay heat and the radioactivity from the fission products (FPs) in the spent fuel mainly depend on the burn-up and the burn-up time rather than the reactor type. Therefore, the decay heat and the radioactivity from FPs in the RMWR spent fuel are smaller, reflecting its relatively long burn-up time resulted from its core characteristics with the high conversion ratio. The radioactivity from the actinides in the spent fuel mainly depends on the {sup 241}Pu content in the initial fuel, and the decay heat mainly depends on {sup 238}Pu and {sup 244}Cm. The contribution of {sup 244}Cm is much smaller in RMWR than in MOX-LWRs because of the difference in the spectrum

LLNL MOX fuel lead assemblies data report for the surplus plutonium disposition environmental impact statement

International Nuclear Information System (INIS)

O'Connor, D.G.; Fisher, S.E.; Holdaway, R.

1998-08-01

The purpose of this document is to support the US Department of Energy (DOE) Fissile Materials Disposition Program's preparation of the draft surplus plutonium disposition environmental impact statement. This is one of several responses to data call requests for background information on activities associated with the operation of the lead assembly (LA) mixed-oxide (MOX) fuel fabrication facility. The DOE Office of Fissile Materials Disposition (DOE-MD) has developed a dual-path strategy for disposition of surplus weapons-grade plutonium. One of the paths is to disposition surplus plutonium through irradiation of MOX fuel in commercial nuclear reactors. MOX fuel consists of plutonium and uranium oxides (PuO 2 and UO 2 ), typically containing 95% or more UO 2 . DOE-MD requested that the DOE Site Operations Offices nominate DOE sites that meet established minimum requirements that could produce MOX LAs. LLNL has proposed an LA MOX fuel fabrication approach that would be done entirely inside an S and S Category 1 area. This includes receipt and storage of PuO 2 powder, fabrication of MOX fuel pellets, assembly of fuel rods and bundles, and shipping of the packaged fuel to a commercial reactor site. Support activities will take place within a Category 1 area. Building 332 will be used to receive and store the bulk PuO 2 powder, fabricate MOX fuel pellets, and assemble fuel rods. Building 334 will be used to assemble, store, and ship fuel bundles. Only minor modifications would be required of Building 332. Uncontaminated glove boxes would need to be removed, petition walls would need to be removed, and minor modifications to the ventilation system would be required

Oxidative dissolution of unirradiated Mimas MOX fuel (U/Pu oxides) in carbonated water under oxic and anoxic conditions

Energy Technology Data Exchange (ETDEWEB)

Odorowski, Mélina [CEA/DEN/DTCD/SECM/LMPA, BP 17171, 30207 Bagnols-sur-Cèze Cedex (France); MINES ParisTech, PSL Research University, Centre de Géosciences, 35 rue St Honoré, 77305 Fontainebleau (France); Jégou, Christophe, E-mail: christophe.jegou@cea.fr [CEA/DEN/DTCD/SECM/LMPA, BP 17171, 30207 Bagnols-sur-Cèze Cedex (France); De Windt, Laurent [MINES ParisTech, PSL Research University, Centre de Géosciences, 35 rue St Honoré, 77305 Fontainebleau (France); Broudic, Véronique; Peuget, Sylvain; Magnin, Magali; Tribet, Magaly [CEA/DEN/DTCD/SECM/LMPA, BP 17171, 30207 Bagnols-sur-Cèze Cedex (France); Martin, Christelle [Agence nationale pour la gestion des déchets radioactifs (Andra), DRD/CM, 1-7 rue Jean-Monnet, 92298 Châtenay-Malabry Cedex (France)

2016-01-15

Few studies exist concerning the alteration of Mimas Mixed-OXide (MOX) fuel, a mixed plutonium and uranium oxide, and data is needed to better understand its behavior under leaching, especially for radioactive waste disposal. In this study, two leaching experiments were conducted on unirradiated MOX fuel with a strong alpha activity (1.3 × 10{sup 9} Bq.g{sub MOX}{sup −1} reproducing the alpha activity of spent MOX fuel with a burnup of 47 GWd·t{sub HM}{sup −1} after 60 years of decay), one under air (oxic conditions) for 5 months and the other under argon (anoxic conditions with [O{sub 2}] < 1 ppm) for one year in carbonated water (10{sup −2} mol L{sup −1}). For each experiment, solution samples were taken over time and Eh and pH were monitored. The uranium in solution was assayed using a kinetic phosphorescence analyzer (KPA), plutonium and americium were analyzed by a radiochemical route, and H{sub 2}O{sub 2} generated by the water radiolysis was quantified by chemiluminescence. Surface characterizations were performed before and after leaching using Scanning Electron Microscopy (SEM), Electron Probe Microanalyzer (EPMA) and Raman spectroscopy. Solubility diagrams were calculated to support data discussion. The uranium releases from MOX pellets under both oxic and anoxic conditions were similar, demonstrating the predominant effect of alpha radiolysis on the oxidative dissolution of the pellets. The uranium released was found to be mostly in solution as carbonate species according to modeling, whereas the Am and Pu released were significantly sorbed or precipitated onto the TiO{sub 2} reactor. An intermediate fraction of Am (12%) was also present as colloids. SEM and EPMA results indicated a preferential dissolution of the UO{sub 2} matrix compared to the Pu-enriched agglomerates, and Raman spectroscopy showed the Pu-enriched agglomerates were slightly oxidized during leaching. Unlike Pu-enriched zones, the UO{sub 2} grains were much more

Advances in Metallic Fuels for High Burnup and Actinide Transmutation

Energy Technology Data Exchange (ETDEWEB)

Hayes, S. L.; Harp, J. M.; Chichester, H. J. M.; Fielding, R. S.; Mariani, R. D.; Carmack, W. J.

2016-10-01

Research and development activities on metallic fuels in the US are focused on their potential use for actinide transmutation in future sodium fast reactors. As part of this application, there is a desire to demonstrate a multifold increase in burnup potential. A number of metallic fuel design innovations are under investigation with a view toward significantly increasing the burnup potential of metallic fuels, since higher discharge burnups equate to lower potential actinide losses during recycle. Promising innovations under investigation include: 1) lowering the fuel smeared density in order to accommodate the additional swelling expected as burnups increase, 2) utilizing an annular fuel geometry for better geometrical stability at low smeared densities, as well as the potential to eliminate the need for a sodium bond, and 3) minor alloy additions to immobilize lanthanide fission products inside the metallic fuel matrix and prevent their transport to the cladding resulting in fuel-cladding chemical interaction. This paper presents results from these efforts to advance metallic fuel technology in support of high burnup and actinide transmutation objectives. Highlights include examples of fabrication of low smeared density annular metallic fuels, experiments to identify alloy additions effective in immobilizing lanthanide fission products, and early postirradiation examinations of annular metallic fuels having low smeared densities and palladium additions for fission product immobilization.

Safeguards on MOX assemblies at LWRs

International Nuclear Information System (INIS)

Arenas Carrasco, J.; Koulikov, I.; Heinonen, O.J.; Arlt, R.; Grigoleit, K.; Clarke, R.; Swinhoe, M.

2000-01-01

Operating within the framework of the New Partnership Approach (NPA) for unirradiated MOX fuel assemblies in LWRs, the IAEA and EURATOM have gained experience in safeguarding 13 LWRs licensed to operate with MOX assemblies. In order to fulfil SIR requirements, verification methods and techniques capable of measuring MOX assemblies under water have been and are still being developed. These encompass both qualitative tests for the detection of plutonium (gross attribute tests) and quantitative tests for the measurement of the amount of plutonium (partial defect tests) and are based on gamma and neutron detection techniques. There are nine PWR and two BWR where the reactor and the spent fuel pond can be covered by the same surveillance device. These are Type I reactors where the reactor and the pond are located in the same hall. In these types of facilities relying on surveillance during the MOX refuelling is especially difficult at the BWRs due to the depth of the core pond. There are two PWR type facilities where the reactor and the spent fuel pond are located in different halls and cannot be covered by the same surveillance device (Type II). An open core camera has not been installed during refuelling and therefore indirect surveillance is currently used to survey MOX loading. Improvements are therefore required and are under consideration. After receipt at the facility, there are a few facilities which must keep the received fresh MOX fuel in wet storage, not only for a short period prior to refuelling, but for more than a year, until the next refuelling campaign. In these cases timely inspections for direct use fresh nuclear material require considerable inspection effort. Additionally, where human surveillance of core loading and finally core closure are necessary there is also a large demand for manpower. Either an agreement should be reached with the operators to delay the MOX loading until the end of the fuelling campaign, or alternative approaches should be

Nuclear fuels with high burnup: safety requirements

International Nuclear Information System (INIS)

Phuc Tran Dai

2016-01-01

Vietnam authorities foresees to build 3 reactors from Russian design (VVER AES 2006) by 2030. In order to prepare the preliminary report on safety analysis the Vietnamese Agency for Radioprotection and Safety has launched an investigation on the behaviour of nuclear fuels at high burnups (up to 60 GWj/tU) that will be those of the new plants. This study deals mainly with the behaviour of the fuel assemblies in case of loss of coolant (LOCA). It appears that for an average burnup of 50 GWj/tU and for the advanced design of the fuel assembly (cladding and materials) safety requirements are fulfilled. For an average burnup of 60 GWj/tU, a list of issues remains to be assessed, among which the impact of clad bursting or the hydrogen embrittlement of the advanced zirconium alloys. (A.C.)

Performance evaluation of WDXRF as a process control technique for MOX fuel fabrication

International Nuclear Information System (INIS)

Pandey, A.; Khan, F.A.; Das, D.K.; Behere, P.G.; Afzal, Mohd

2015-01-01

This paper presents studies on Wavelength Dispersive X-Ray Fluorescence (WDXRF), as a powerful non destructive technique (NDT) for the compositional analysis of various types of MOX fuels. The sample has come after mixing and milling of UO 2 and PuO 2 powder for the estimation of plutonium, as a process control step of fabrication of (U, Pu)O 2 mixed oxide (MOX) fuel. For the characterization for heavy metal in various MOX fuel, a WDXRF method was established as a process control technique. The attractiveness of our system is that it can analyze the samples in solid form as well as in liquid form. The system is adapted in a glove box for handling of plutonium based fuels. The glove box adapted system was optimized with Uranium and Thorium based MOX sample before introduction of Pu. Uranium oxide and thorium oxide have been estimated in uranium thorium MOX samples. Standard deviation for the analysis of U 3 O 8 and ThO 2 were found to be 0.14 and 0.15 respectively. The results are validated against the conventional wet chemical methods of analysis. (author)

Mixed-oxide (MOX) fuel performance benchmark. Summary of the results for the PRIMO MOX rod BD8

International Nuclear Information System (INIS)

Ott, L.J.; Sartori, E.; Costa, A.; ); Sobolev, V.; Lee, B-H.; Alekseev, P.N.; Shestopalov, A.A.; Mikityuk, K.O.; Fomichenko, P.A.; Shatrova, L.P.; Medvedev, A.V.; Bogatyr, S.M.; Khvostov, G.A.; Kuznetsov, V.I.; Stoenescu, R.; Chatwin, C.P.

2009-01-01

The OECD/NEA Nuclear Science Committee has established an Expert Group that deals with the status and trends of reactor physics, nuclear fuel performance, and fuel cycle issues related to the disposition of weapons-grade plutonium as MOX fuel. The activities of the NEA Expert Group on Reactor-based Plutonium Disposition are carried out in close cooperation with the NEA Working Party on Scientific Issues in Reactor Systems (WPRS). A major part of these activities includes benchmark studies. This report describes the results of the PRIMO rod BD8 benchmark exercise, the second benchmark by the TFRPD relative to MOX fuel behaviour. The corresponding PRIMO experimental data have been released, compiled and reviewed for the International Fuel Performance Experiments (IFPE) database. The observed ranges (as noted in the text) in the predicted thermal and FGR responses are reasonable given the variety and combination of thermal conductivity and FGR models employed by the benchmark participants with their respective fuel performance codes

Fuel assembly

International Nuclear Information System (INIS)

Fushimi, Atsushi; Shimada, Hidemitsu; Aoyama, Motoo; Nakajima, Junjiro

1998-01-01

In a fuel assembly for an n x n lattice-like BWR type reactor, n is determined to 9 or greater, and the enrichment degree of plutonium is determined to 4.4% by weight or less. Alternatively, n is determined to 10 or greater, and the enrichment degree of plutonium is determined to 5.2% by weight or less. An average take-out burnup degree is determined to 39GWd/t or less, and the matrix is determined to 9 x 9 or more, or the average take-out burnup degree is determined to 51GWd/t, and the matrix is determined to 10 x 10 or more and the increase of the margin of the maximum power density obtained thereby is utilized for the compensation of the increase of distortion of power distribution due to decrease of the kinds of plutonium enrichment degree, thereby enabling to reduce the kind of the enrichment degree of MOX fuel rods to one. As a result, the manufacturing step for fuel pellets can be simplified to reduce the manufacturing cost for MOX fuel assemblies. (N.H.)

Conceptual study of the future nuclear fuel cycle system for the extended LWR age

International Nuclear Information System (INIS)

Fujine, Sachio; Takano, Hideki; Sato, Osamu; Tone, Tatsuzo; Yamada, Takashi; Kurosawa, Katsutoshi.

1993-08-01

A large scale integrated fuel cycle facility (IFCF) is assumed for the future nuclear fuel cycle in the extended LWR age. Spent MOX fuels are reprocessed mixed with UOX in a centralized reprocessing plant. The reprocessing plant separates long-lived nuclides as well as Pu. Nitric acid solutions of those products are fed directly to MOX fabrication process which is incorporated with reprocessing. MOX pellets are made by sphere-cal process. Two process concepts are made as advanced reprocessing incorporated with partitioning (ARP) which has the function of long-lived nuclides recovery. One is a simplified Purex combined with partitioning. Extractable long-lived nuclides, 237 Np and 99 Tc, are assumed to be recovered in main flow stream of the improved Purex process. The other process concept is made aiming at recovering all TRU nuclides in reprocessing to meet with TRU recycle requirement in the long future. A concept of the future fuel cycle system is made by combining integrated fuel cycle facility and very high burnup LWRs (VHBR). The reactor concept of VHBRs has been proposed to improve Pu recycle economy in the future. Highly enriched MOX fuel are loaded in the full core of reactor in order to increase reactivity for the burnup. Fuel cycle indices such as Pu isotopic composition change, spent fuel integration, nuclide transmutation effect are estimated by simulating the Pu recycling in the system of VHBR and ARP. It is concluded that Pu enrichment of MOX fuel can be kept less than 20 % through multi-recycle. Reprocessing MOX fuels with UOX shows a favorable effect for keeping Pu reactivity high enough for VHBR. Integration of spent MOX fuel can be reduced by Pu recycle. Transmutation of Np is feasible by containing Np into MOX fuel. (author)

Technical Issues in the development of high burnup and long cycle fuel pellets

Energy Technology Data Exchange (ETDEWEB)

Kim, Dong Joo; Yang, Jae Ho; Oh, Jang Soo; Kim, Keon Sik; Rhee, Young Woo; Kim, Jong Hun; Nam, Ik Hui [Korea Atomic Energy Research Institute, Daejeon (Korea, Republic of)

2012-10-15

Over the last half century, a nuclear fuel cycle, a fuel discharged burnup and a uranium enrichment of the LWR (Light Water Reactor) fuel have continuously increased. It was the efforts to reduce the LWR fuel cycle cost, and to make reactor operation more efficiently. Improved fuel and reactor performance contribute further to the reduction and management efficiency of spent fuels. The primary incentive for operating nuclear reactor fuel to higher burnup and longer cycle is the economic benefits. The fuel cycle costs could be reduced by extending fuel discharged burnup and fuel cycle length. The higher discharged burnup can increase the energy production per unit fuel mass or fuel assembly. The longer fuel cycle can increase reactor operation flexibility and reduce the fuel changing operation and the spent fuel management burden. The margin to storage capacity limits would be also increased because high burnup and long cycle fuel reduces the mass of spent fuels. However, increment of fuel burnup and cycle length might result in the acceleration of material aging consisting fuel assembly. Then, the safety and integrity of nuclear fuel will be degraded. Therefore, to simultaneously enhance the safety and economics of the LWR fuel through the fuel burnup and cycle extension, it is indispensable to develop the innovative nuclear fuel material concepts and technologies which can overcome degradation of fuel safety. New fuel research project to extend fuel discharged burnup and cycle length has been launched in KAERI. Main subject is to develop innovative LWR fuel pellets which can provide required fuel performance and safety at extended fuel burnup and cycle length. In order to achieve the mission, we need to know that what the impediments are and how to break through current limit of fuel pellet properties. In this study, the technical issues related to fuel pellets at high burnup were surveyed and summarized. We have collected the technical issues in the literatures

Technical Issues in the development of high burnup and long cycle fuel pellets

International Nuclear Information System (INIS)

Kim, Dong Joo; Yang, Jae Ho; Oh, Jang Soo; Kim, Keon Sik; Rhee, Young Woo; Kim, Jong Hun; Nam, Ik Hui

2012-01-01

Over the last half century, a nuclear fuel cycle, a fuel discharged burnup and a uranium enrichment of the LWR (Light Water Reactor) fuel have continuously increased. It was the efforts to reduce the LWR fuel cycle cost, and to make reactor operation more efficiently. Improved fuel and reactor performance contribute further to the reduction and management efficiency of spent fuels. The primary incentive for operating nuclear reactor fuel to higher burnup and longer cycle is the economic benefits. The fuel cycle costs could be reduced by extending fuel discharged burnup and fuel cycle length. The higher discharged burnup can increase the energy production per unit fuel mass or fuel assembly. The longer fuel cycle can increase reactor operation flexibility and reduce the fuel changing operation and the spent fuel management burden. The margin to storage capacity limits would be also increased because high burnup and long cycle fuel reduces the mass of spent fuels. However, increment of fuel burnup and cycle length might result in the acceleration of material aging consisting fuel assembly. Then, the safety and integrity of nuclear fuel will be degraded. Therefore, to simultaneously enhance the safety and economics of the LWR fuel through the fuel burnup and cycle extension, it is indispensable to develop the innovative nuclear fuel material concepts and technologies which can overcome degradation of fuel safety. New fuel research project to extend fuel discharged burnup and cycle length has been launched in KAERI. Main subject is to develop innovative LWR fuel pellets which can provide required fuel performance and safety at extended fuel burnup and cycle length. In order to achieve the mission, we need to know that what the impediments are and how to break through current limit of fuel pellet properties. In this study, the technical issues related to fuel pellets at high burnup were surveyed and summarized. We have collected the technical issues in the literatures

Burnup credit feasibility for BWR spent fuel shipments

International Nuclear Information System (INIS)

Broadhead, B.L.

1990-01-01

Considerable interest in the allowance of reactivity credit for the exposure history of power reactor fuel currently exists. This ''burnup credit'' issue has the potential to greatly reduce risk and cost when applied to the design and certification of spent of fuel casks used for transportation and storage. Analyses 1 have shown the feasibility estimated the risk and economic incentives for allowing burnup credit in pressurized water reactor (PWR) spent fuel shipping cask applications. This paper summarizes the extension of the previous PWR feasibility assessments to boiling water reactor (BWR) fuel. As with the PWR analysis, the purpose was not verification of burnup credit (see ref. 2 for ongoing work in this area) but a reasonable assessment of the feasibility and potential gains from its use in BWR applications. This feasibility analysis aims to apply simple methods that adequately characterize the time-dependent isotopic compositions of typical BWR fuel. An initial analysis objective was to identify a simple and reliable method for characterizing BWR spent fuel. The method includes characterization of a typical pin-cell spectrum, using a one-dimensional (1-D) model of a BWR assembly. The calculated spectrum allows burnup-dependent few-group material constants to be generated. Point depletion methods were then used to obtain the time-varying characteristics of the fuel. These simple methods were validated, where practical, with multidimensional methods. 6 refs., 1 tab

LLNL MOX fuel lead assemblies data report for the surplus plutonium disposition environmental impact statement

Energy Technology Data Exchange (ETDEWEB)

O`Connor, D.G.; Fisher, S.E.; Holdaway, R. [and others

1998-08-01

The purpose of this document is to support the US Department of Energy (DOE) Fissile Materials Disposition Program`s preparation of the draft surplus plutonium disposition environmental impact statement. This is one of several responses to data call requests for background information on activities associated with the operation of the lead assembly (LA) mixed-oxide (MOX) fuel fabrication facility. The DOE Office of Fissile Materials Disposition (DOE-MD) has developed a dual-path strategy for disposition of surplus weapons-grade plutonium. One of the paths is to disposition surplus plutonium through irradiation of MOX fuel in commercial nuclear reactors. MOX fuel consists of plutonium and uranium oxides (PuO{sub 2} and UO{sub 2}), typically containing 95% or more UO{sub 2}. DOE-MD requested that the DOE Site Operations Offices nominate DOE sites that meet established minimum requirements that could produce MOX LAs. LLNL has proposed an LA MOX fuel fabrication approach that would be done entirely inside an S and S Category 1 area. This includes receipt and storage of PuO{sub 2} powder, fabrication of MOX fuel pellets, assembly of fuel rods and bundles, and shipping of the packaged fuel to a commercial reactor site. Support activities will take place within a Category 1 area. Building 332 will be used to receive and store the bulk PuO{sub 2} powder, fabricate MOX fuel pellets, and assemble fuel rods. Building 334 will be used to assemble, store, and ship fuel bundles. Only minor modifications would be required of Building 332. Uncontaminated glove boxes would need to be removed, petition walls would need to be removed, and minor modifications to the ventilation system would be required.

Investigation of Burnup Credit Issues in BWR Fuel

International Nuclear Information System (INIS)

Broadhead, B.L.; DeHart, M.D.

1999-01-01

Calculations for long-term-disposal criticality safety of spent nuclear fuel requires the application of burnup credit because of the large mass of fissile material that will be present in the repository. Burnup credit calculations are based on depletion calculations that provide a conservative estimate of spent fuel contents, followed by criticality calculations to assess the value of keff for a spent fuel cask or a fuel configuration under a variety of probabilistically derived events. In order to ensure that the depletion calculation is conservative, it is necessary to both qualify and quantify assumptions that can be made in depletion models used to characterize spent fuel. Most effort in the United States this decade has focused on burnup issues related to pressurized-water reactors. However, requirements for the permanent disposal of fuel from boiling-water reactors has necessitated development of methods for prediction of spent fuel contents for such fuels. Concomitant with such analyses, validation is also necessary. This paper provides a summary of initial efforts at the Oak Ridge National Laboratory to better understand and validate spent fuel analyses for boiling-water-reactor fuel

Extended burnup with SEU fuel in Atucha-1 NPP

International Nuclear Information System (INIS)

Alvarez, L.; Casario, J.; Fink, J.; Perez, R.; Higa, M.

2002-01-01

Atucha-1 is a Pressurized Heavy Water Reactor originally fuelled with natural uranium. Fuel Assemblies consist of 36 fuel rods and the active length is 5300 mm. The total length of the fuel assembly is about 6 m. The average discharge burnup of natural UO 2 fuel is 5900 MWd/tU. After the deregulation of the Argentine electricity market there was an important incentive to reduce the impact of fuel cost on the cost of generation. To keep the competitiveness of the nuclear energy against another sources of electricity it was necessary to reduce the cost of the nuclear fuel. With this objective a program to introduce SEU (0.85 % 235 U) fuel in Atucha-1 was launched in 1993. As a result of this program the average SEU fuel discharge burnup increased to more than 11000 MWd/tU. The first SEU fuels were introduced in Atucha-1 in 1995 and, in the present stage of the program, 71% of core positions are loaded with this type of fuel. This paper describes key aspects of Atucha-1 fuel design and their relevance limiting the burnup extension and shows relevant data regarding the SEU in-reactor performance. At the present time 125 SEU Fuel Assemblies have been irradiated without failures associated with the extended burnup or unfavorable influences on the operation of the power station. (author)

Development of moderated neutron calibration fields simulating workplaces of MOX fuel facilities

International Nuclear Information System (INIS)

Tsujimura, Norio; Yoshida, Tadayoshi; Takada, Chie

2005-01-01

It is important for the MOX fuel facilities to control neutrons produced by the spontaneous fission of plutonium isotopes and those from (α,n) reactions between 18 O and α particles emitted by 238 Pu. Neutron dose meters should be calibrated for measuring these neutrons. We have developed moderated-neutron calibration fields employing a 252 Cf neutron source and moderators mainly for the characteristics evaluation and the calibration of neutron detectors used in MOX fuel facilities. Neutron energy spectrum can be adjusted by changing the position of the 252 Cf neutron source and combining different moderators to simulate the neutron field of the MOX fuel facility. This performance is realized owing to using an existing neutron irradiation room. (K. Yoshida)

Discharge Burnup Evaluation of Natural Uranium Loaded CANFLEX-43 Fuel Bundle

International Nuclear Information System (INIS)

Roh, Gyu Hong; Kim, Yong Hee; Kim, Won Young; Park, Joo Hwan

2009-11-01

Using WIMS-AECL code, which is 2-dimensional lattice core used in CANDU physics calculation, the discharge burnup of the natural uranium loaded CANFLEX-43 fuel bundle was evaluated by comparing the discharge burnup of standard 37 element fuel bundle. When the discharge burnup of the standard 37 element fuel is 7,200 MWd/MTU, that of the CANFLEX 43 fuel bundle was evaluated as 7,077 MWd/MTU, by applying the same lattice conditions for both fuel bundles

Technical Development on Burn-up Credit for Spent LWR Fuel

Energy Technology Data Exchange (ETDEWEB)

Gauld, I.C.

2001-12-26

Technical development on burn-up credit for spent LWR fuels had been performed at JAERI since 1990 under the contract with Science and Technology Agency of Japan entitled ''Technical Development on Criticality Safety Management for Spent LWR Fuels.'' Main purposes of this work are to obtain the experimental data on criticality properties and isotopic compositions of spent LWR fuels and to verify burnup and criticality calculation codes. In this work three major experiments of exponential experiments for spent fuel assemblies to obtain criticality data, non-destructive gamma-ray measurement of spent fuel rods for evaluating axial burn-up profiles, and destructive analyses of spent fuel samples for determining precise burn-up and isotopic compositions were carried out. The measured data obtained were used for validating calculation codes as well as an examination of criticality safety analyses. Details of the work are described in this report.

Technical development on burn-up credit for spent LWR fuels

International Nuclear Information System (INIS)

Nakahara, Yoshinori; Suyama, Kenya; Suzaki, Takenori

2000-10-01

Technical development on burn-up credit for spent LWR fuels had been performed at JAERI since 1990 under the contract with Science and Technology Agency of Japan entitled 'Technical Development on Criticality Safety Management for Spent LWR Fuels'. Main purposes of this work are to obtain the experimental data on criticality properties and isotopic compositions of spent LWR fuels and to verify burn-up and criticality calculation codes. In this work three major experiments of exponential experiments for spent fuel assemblies to obtain criticality data, non-destructive gamma-ray measurement of spent fuel rods for evaluating axial burn-up profiles, and destructive analyses of spent fuel samples for determining precise burn-up and isotopic compositions were carried out. The measured data obtained were used for validating calculation codes as well as an examination of criticality safety analyses. Details of the work are described in this report. (author)

Technical development on burn-up credit for spent LWR fuels

Energy Technology Data Exchange (ETDEWEB)

Nakahara, Yoshinori; Suyama, Kenya; Suzaki, Takenori [eds.] [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

2000-10-01

Technical development on burn-up credit for spent LWR fuels had been performed at JAERI since 1990 under the contract with Science and Technology Agency of Japan entitled 'Technical Development on Criticality Safety Management for Spent LWR Fuels'. Main purposes of this work are to obtain the experimental data on criticality properties and isotopic compositions of spent LWR fuels and to verify burn-up and criticality calculation codes. In this work three major experiments of exponential experiments for spent fuel assemblies to obtain criticality data, non-destructive gamma-ray measurement of spent fuel rods for evaluating axial burn-up profiles, and destructive analyses of spent fuel samples for determining precise burn-up and isotopic compositions were carried out. The measured data obtained were used for validating calculation codes as well as an examination of criticality safety analyses. Details of the work are described in this report. (author)

Safety aspects related to burnup increase and mixed oxide fuel

International Nuclear Information System (INIS)

Thomas, W.

1992-01-01

The dominant factor presently limiting the fuel burnup is the response of the cladding hulls. To maintain the excellent record of very low fuel failure rates for increased burnups further technical development is underway and necessary. In the nuclear fuel cycle increased burnups lead to a remarkable reduction of spent fuel arisings and corresponding economic savings. Thermal recycling of plutonium presently provides an opportunity to reduce the rising accumulation of plutunium in a situation where there is no demand for this fissile material in Fast Breeder Reactors. (orig.) [de

Development and validation of the ENIGMA code for MOX fuel performance modelling

International Nuclear Information System (INIS)

Palmer, I.; Rossiter, G.; White, R.J.

2000-01-01

The ENIGMA fuel performance code has been under development in the UK since the mid-1980s with contributions made by both the fuel vendor (BNFL) and the utility (British Energy). In recent years it has become the principal code for UO 2 fuel licensing for both PWR and AGR reactor systems in the UK and has also been used by BNFL in support of overseas UO 2 and MOX fuel business. A significant new programme of work has recently been initiated by BNFL to further develop the code specifically for MOX fuel application. Model development is proceeding hand in hand with a major programme of MOX fuel testing and PIE studies, with the objective of producing a fuel modelling code suitable for mechanistic analysis, as well as for licensing applications. This paper gives an overview of the model developments being undertaken and of the experimental data being used to underpin and to validate the code. The paper provides a summary of the code development programme together with specific examples of new models produced. (author)

A review on the development of the MOX fuel fabrication technology

Energy Technology Data Exchange (ETDEWEB)

Kim, See Hyung; Lee, Yung Woo; Sohn, Dong Sung; Yang, Myung Seung; Bae, Kee Kwang; Nah, Sang Hoh; Kim, Han Soo; Lee, Jung Won; Kim, Bong Koo; Song, Keun Woo [Korea Atomic Energy Research Institute, Taejon (Korea, Republic of)

1995-07-01

Development of the Mixed Oxide(MOX) fuel fabrication technology was reviewed in this study. Firstly, the feasibility of Pu utilization for nuclear fuel was analyzed by comparison of nuclear characteristics between U and Pu. Secondly, the feature and problem of processes developed so far was revealed and analyzed by reviewing each process in terms of technical difficulties and in connection with the pellet characteristics. Also, fabrication facilities currently existing were analyzed to understand particularities and circumstances in view of Pu handling, and finally, in-reactor behaviors of MOX fuel was compared with those of U fuel to understand how the Pu has an effect on fuel was compared with those of U fuel to understand how the Pu has an effect on fuel pellet structure and fuel rod. 73 figs., 15 tabs., 58 refs. (Author).

Transportation and packaging issues involving the disposition of surplus plutonium as MOX fuel in commercial LWRs

International Nuclear Information System (INIS)

Ludwig, S.B.; Welch, D.E.; Best, R.E.; Schmid, S.P.

1997-08-01

This report provides a view of anticipated transportation, packaging, and facility handling operations that are expected to occur at mixed-oxide (MOX) fuel fabrication and commercial reactor facilities. This information is intended for use by prospective contractors to the U.S. Department of Energy (DOE) who plan to submit proposals to DOE to manufacture and irradiate MOX fuel assemblies in domestic commercial light-water reactors. The report provides data to prospective consortia regarding packaging and pickup of MOX nuclear fuel assemblies at a MOX fuel manufacturing plant and transport and delivery of the MOX assemblies to nuclear power plants. The report also identifies areas where data are incomplete either because of the status of development or lack of sufficient information and specificity regarding the nuclear power plant(s) where deliveries will take place

Implementation of burnup credit in spent fuel management systems

International Nuclear Information System (INIS)

Dyck, H.P.

2001-01-01

Improved calculational methods allow one to take credit for the reactivity reduction associated with fuel burnup. This means reducing the analysis conservatism while maintaining an adequate safety margin. The motivation for using burnup credit in criticality safety applications is based on economic considerations and additional benefits contributing to public health and safety and resource conservation. Interest in the implementation of burnup credit has been shown by many countries. In 1997, the International Atomic Energy Agency (IAEA) started a task to monitor the implementation of burnup credit in spent fuel management systems, to provide a forum to exchange information, to discuss the matter and to gather and disseminate information on the status of national practices of burnup credit implementation in the Member States. The task addresses current and future aspects of burnup credit. This task was continued during the following years. (author)

Fuel cycle cost considerations of increased discharge burnups

International Nuclear Information System (INIS)

Scherpereel, L.R.; Frank, F.J.

1982-01-01

Evaluations are presented that indicate the attainment of increased discharge burnups in light water reactors will depend on economic factors particular to individual operators. In addition to pure resource conserving effects and assuming continued reliable fuel performance, a substantial economic incentive must exist to justify the longer operating times necessary to achieve higher burnups. Whether such incentive will exist or not will depend on relative price levels of all fuel cycle cost components, utility operating practices, and resolution of uncertainties associated with the back-end of the fuel cycle. It is concluded that implementation of increased burnups will continue at a graduated pace similar to past experience, rather than finding universal acceptance of particular increased levels at any particular time

Simulation of facility operations and materials accounting for a combined reprocessing/MOX fuel fabrication facility

International Nuclear Information System (INIS)

Coulter, C.A.; Whiteson, R.; Zardecki, A.

1991-01-01

We are developing a computer model of facility operations and nuclear materials accounting for a facility that reprocesses spent fuel and fabricates mixed oxide (MOX) fuel rods and assemblies from the recovered uranium and plutonium. The model will be used to determine the effectiveness of various materials measurement strategies for the facility and, ultimately, of other facility safeguards functions as well. This portion of the facility consists of a spent fuel storage pond, fuel shear, dissolver, clarifier, three solvent-extraction stages with uranium-plutonium separation after the first stage, and product concentrators. In this facility area mixed oxide is formed into pellets, the pellets are loaded into fuel rods, and the fuel rods are fabricated into fuel assemblies. These two facility sections are connected by a MOX conversion line in which the uranium and plutonium solutions from reprocessing are converted to mixed oxide. The model of the intermediate MOX conversion line used in the model is based on a design provided by Mike Ehinger of Oak Ridge National Laboratory (private communication). An initial version of the simulation model has been developed for the entire MOX conversion and fuel fabrication sections of the reprocessing/MOX fuel fabrication facility, and this model has been used to obtain inventory difference variance estimates for those sections of the facility. A significant fraction of the data files for the fuel reprocessing section have been developed, but these data files are not yet complete enough to permit simulation of reprocessing operations in the facility. Accordingly, the discussion in the following sections is restricted to the MOX conversion and fuel fabrication lines. 3 tabs

Modelling of phenomena associated with high burnup fuel behaviour during overpower transients

International Nuclear Information System (INIS)

Sills, H.E.; Langman, V.J.; Iglesias, F.C.

1995-01-01

Phenomena of importance to the behaviour of high burnup fuel subjected to conditions of rapid overpower (i.e., LWR RIAs) include the change in cladding material properties due to irradiation, pellet-clad interaction (PCI) and 'rim' effects associated with the periphery of high burnup fuel. 'Rim' effects are postulated to be caused by changes in fuel morphology at high burnup. Typical discharge burnups for CANDU fuel are low compared to LWRs. Maximum linear ratings for CANDU fuel are higher than those for LWRs. However, under normal operating conditions, the Zircaloy-4 clad of the CANDU fuel is collapsed onto the fuel stack. Thus, the CANDU fuel performance codes model the transient behaviour of the fuel-to-clad interface and are capable of assessing the potential for pellet-clad mechanical interaction (PCMI) failures for a wide range of overpower conditions. This report provides a discussion of the modelling of the phenomena of importance to high burnup fuel behaviour during rapid overpower transients. (author)

TRIGA fuel element burnup determination by measurement and calculation

International Nuclear Information System (INIS)

Zagar, T.; Ravnik, M.; Persic, A.; Jeraj, R.

2000-01-01

To estimate the accuracy of the fuel element burnup calculation different factors influencing the calculation were studied. To cover different aspects of burnup calculations, two in-house developed computer codes were used in calculations. The first (TRIGAP) is based on a one-dimensional two-group diffusion approximation, and the second (TRIGLAV) is based on a two-dimensional four-group diffusion equation. Both codes use WIMSD program with different libraries forunit-cell cross section data calculation. The burnup accumulated during the operating history of the TRIGA reactor at Josef Stefan Institute was calculated for all fuel elements. Elements used in the core during this period were standard SS 8.5% fuel elements, standard SS 12% fuel elements and highly enriched FLIP fuel elements. During the considerable period of operational history, FLIP and standard fuel elements were used simultaneously in mixed cores. (authors)

The Gd-isotopic fuel for high burnup in PWR's

International Nuclear Information System (INIS)

Dias, Marcio Soares; Mattos, João Roberto L. de; Andrade, Edison Pereira de

2017-01-01

Today, the discussion about the high burnup fuel is beyond the current fuel enrichment licensing and burnup limits. Licensing issues and material/design developments are again key features in further development of the LWR fuel design. Nevertheless, technological and economical solutions are already available or will be available in a short time. In order to prevent the growth of the technological gap, Brazil's nuclear sector needs to invest in the training of new human resources, in the access to international databases, and in the upgrading existing infrastructure. Experimental database and R&D infrastructure are essential components to support the autonomous development of Brazilian Nuclear Reactors, promoting the development of national technologies. The (U,Gd)O_2 isotopic fuel proposed by the CDTN's staff solve two main issues in the high burnup fuel, which are (1) the peak of reactivity resulting from the Gd-157 fast burnup, and (2) the peak of temperature in the (U,Gd)O_2 nuclear fuel resulting from detrimental effects in the thermal properties for gadolinia additions higher than 2%. A sustainable future can be envisaged for the nuclear energy. (author)

Fuel element burnup measurements for the equilibrium LEU silicide RSG GAS (MPR-30) core under a new fuel management strategy

International Nuclear Information System (INIS)

Pinem, Surian; Liem, Peng Hong; Sembiring, Tagor Malem; Surbakti, Tukiran

2016-01-01

Highlights: • Burnup measurement of fuel elements comprising the new equilibrium LEU silicide core of RSG GAS. • The burnup measurement method is based on a linear relationship between reactivity and burnup. • Burnup verification was conducted using an in-house, in-core fuel management code BATAN-FUEL. • A good agreement between the measured and calculated burnup was confirmed. • The new fuel management strategy was confirmed and validated. - Abstract: After the equilibrium LEU silicide core of RSG GAS was achieved, there was a strong need to validate the new fuel management strategy by measuring burnup of fuel elements comprising the core. Since the regulatory body had a great concern on the safety limit of the silicide fuel element burnup, amongst the 35 burnt fuel elements we selected 22 fuel elements with high burnup classes i.e. from 20 to 53% loss of U-235 (declared values) for the present measurements. The burnup measurement method was based on a linear relationship between reactivity and burnup where the measurements were conducted under subcritical conditions using two fission counters of the reactor startup channel. The measurement results were compared with the declared burnup evaluated by an in-house in-core fuel management code, BATAN-FUEL. A good agreement between the measured burnup values and the calculated ones was found within 8% uncertainties. Possible major sources of differences were identified, i.e. large statistical errors (i.e. low fission counters’ count rates), variation of initial U-235 loading per fuel element and accuracy of control rod indicators. The measured burnup of the 22 fuel elements provided the confirmation of the core burnup distribution planned for the equilibrium LEU silicide core under the new fuel management strategy.

Ultrasonic measurement of high burn-up fuel elastic properties

International Nuclear Information System (INIS)

Laux, D.; Despaux, G.; Augereau, F.; Attal, J.; Gatt, J.; Basini, V.

2006-01-01

The ultrasonic method developed for the evaluation of high burn-up fuel elastic properties is presented hereafter. The objective of the method is to provide data for fuel thermo-mechanical calculation codes in order to improve industrial nuclear fuel and materials or to design new reactor components. The need for data is especially crucial for high burn-up fuel modelling for which the fuel mechanical properties are essential and for which a wide range of experiments in MTR reactors and high burn-up commercial reactor fuel examinations have been included in programmes worldwide. To contribute to the acquisition of this knowledge the LAIN activity is developing in two directions. First one is development of an ultrasonic focused technique adapted to active materials study. This technique was used few years ago in the EdF laboratory in Chinon to assess the ageing of materials under irradiation. It is now used in a hot cell at ITU Karlsruhe to determine the elastic moduli of high burnup fuels from 0 to 110 GWd/tU. Some of this work is presented here. The second on going programme is related to the qualification of acoustic sensors in nuclear environments, which is of a great interest for all the methods, which work, in a hostile nuclear environment

Full MOX core design in ABWR

International Nuclear Information System (INIS)

Ihara, Toshiteru; Mochida, Takaaki; Izutsu, Sadayuki; Fujimaki, Shingo

2003-01-01

Electric Power Development Co., Ltd. (EPDC) has been investigating an ABWR plant for construction at Oma-machi in Aomori Prefecture. The reactor, termed FULL MOX-ABWR will have its reactor core eventually loaded entirely with mixed-oxide (MOX) fuel. Extended use of MOX fuel in the plant is expected to play important roles in the country's nuclear fuel recycling policy. MOX fuel bundles will initially be loaded only to less than one-third of the reactor, but will be increased to cover its entire core eventually. The number of MOX fuel bundles in the core thus varies anywhere from 0 to 264 for the initial cycle and, 0 to 872 for equilibrium cycles. The safety design of the FULL MOX-ABWR briefly stated next considers any probable MOX loading combinations out of such MOX bundle usage scheme, starting from full UO 2 to full MOX cores. (author)

Fuel element burnup determination in HEU-LEU mixed TRIGA research reactor core

International Nuclear Information System (INIS)

Zagar, Tomaz; Ravnik, Matjaz

2000-01-01

This paper presents the results of a burnup calculations and burnup measurements for TRIGA FLIP HEU fuel elements and standard TRIGA LEU fuel elements used simultaneously in small TRIGA Mark II research reactor in Ljubljana, Slovenija. The fuel element burnup for approximately 15 years of operation was calculated with two different in house computer codes TRIGAP and TRIGLAV (both codes are available at OECD NEA Data Bank). The calculation is performed in one-dimensional radial geometry in TRIGAP and in two-dimensional (r,φ) geometry in TRIGLAV. Inter-comparison of results shows important influence of in-core water gaps, irradiation channels and mixed rings on burnup calculation accuracy. Burnup of 5 HEU and 27 LEU fuel elements was also measured with reactivity method. Measured and calculated burnup values are inter-compared for these elements (author)

IAEA activities in the back-end area of nuclear fuel cycle

International Nuclear Information System (INIS)

Fukuda, Kosaku

1999-01-01

This paper concerns recent outcomes from the IAEA's activities in the area of the nuclear fuel cycle, particularly focusing on the back-end of the fuel cycle. It includes spent fuel management, plutonium utilization and burnup credit. In the area of spent fuel management, worldwide prospects and status of the spent fuel arising, storage and reprocessing are presented. In the area of plutonium utilization worldwide, only MOX fuel fabrication is described. Finally, the worldwide status of the burnup credit implementation is described. (author)

Performance of the MTR core with MOX fuel using the MCNP4C2 code

International Nuclear Information System (INIS)

Shaaban, Ismail; Albarhoum, Mohamad

2016-01-01

The MCNP4C2 code was used to simulate the MTR-22 MW research reactor and perform the neutronic analysis for a new fuel namely: a MOX (U 3 O 8 &PuO 2 ) fuel dispersed in an Al matrix for One Neutronic Trap (ONT) and Three Neutronic Traps (TNTs) in its core. Its new characteristics were compared to its original characteristics based on the U 3 O 8 -Al fuel. Experimental data for the neutronic parameters including criticality relative to the MTR-22 MW reactor for the original U 3 O 8 -Al fuel at nominal power were used to validate the calculated values and were found acceptable. The achieved results seem to confirm that the use of MOX fuel in the MTR-22 MW will not degrade the safe operational conditions of the reactor. In addition, the use of MOX fuel in the MTR-22 MW core leads to reduce the uranium fuel enrichment with 235 U and the amount of loaded 235 U in the core by about 34.84% and 15.21% for the ONT and TNTs cases, respectively. - Highlights: • Re-cycling of the ETRR-2 reactor by MOX fuel. • Increase the number of the neutronic traps from one neutronic trap to three neutronic trap. • Calculation of the criticality safety and neutronic parameters of the ETRR-2 reactor for the U 3 O 8 -Al original fuel and the MOX fuel.

Burnup measurements of leader fuel elements

International Nuclear Information System (INIS)

Henriquez, C; Navarro, G; Pereda, C

2000-01-01

Some time ago the CCHEN authorities decided to produce a set of 50 low enrichment fuel elements. These elements were produced in the PEC (Fuel Elements Plant), located at CCHEN offices in Lo Aguirre. These new fuel elements have basically the same geometrical characteristics of previous ones, which were British and made with raw material from the U.S. The principal differences between our fuel elements and the British ones is the density of fissile material, U-235, which was increased to compensate the reduction in enrichment. Last year, the Fuel Elements Plant (PEC) delivered the shipment's first four (4) fuel elements, called leaders, to the RECH1. A test element was delivered too, and the complete set was introduced into the reactor's nucleus, following the normal routine, but performing a special follow-up on their behavior inside the nucleus. This experimental element has only one outside fuel plate, and the remaining (15) structural plates are aluminum. In order to study the burnup, the test element was taken out of the nucleus, in mid- November 1999, and left to decay until June 2000, when it was moved to the laboratory (High Activity Cell), to start the burnup measurements, with a gamma spectroscopy system. This work aims to show the results of these measurements and in addition to meet the following objectives: (a) Visual test of the plate's general condition; (b) Sipping test of fission products; (c) Study of burn-up distribution in the plate; (d) Check and improve the calculus algorithm; (e) Comparison of the results obtained from the spectroscopy with the ones from neutron calculus

Determination of burn-up of irradiated nuclear fuels using mass spectrometry

International Nuclear Information System (INIS)

Jagadish Kumar, S.; Telmore, V.M.; Shah, R.V.; Sasi Bhushan, K.; Paul, Sumana; Kumar, Pranaw; Rao, Radhika M.; Jaison, P.G.

2017-01-01

Burn-up defined as the atom percent fission, is a vital parameter used for assessing the performance of nuclear fuel during its irradiation in the reactor. Accurate data on the actinide isotopes are also essential for the reliable accountability of nuclear materials and for nuclear safeguards. Both destructive and non-destructive methods are employed in the post-irradiation analysis for the burn-up measurements. Though non-destructive methods are preferred from the point view of remote handling of irradiated fuels with high radioactivity, they do not provide the high accuracy as achieved by the chemical analysis methods. Thus destructive radiochemical and chemical analyses are still the established reference methods for accurate and reliable burn-up determination of irradiated nuclear fuels. In the destructive method, burn-up of irradiated nuclear fuel is determined by correlating the amount of a fission product formed during irradiation with that of heavy elements. Thus the destructive experimental determination of burn-up involves the dissolution of irradiated fuel samples followed by the separation and determination of heavy elements and fission product(s) to be used as burn-up monitor(s). Another approach for the experimental determination of burn-up is based on the changes in the abundances of the heavy element isotopes. A widely accepted method for burn-up determination is based on stable "1"4"8Nd and "1"3"9La as burn-up monitors. Several properties such as non-volatility, nearly same yields for thermal fissions of "2"3"5U and "2"3"9Pu etc justifies the selection of "1"4"8Nd as a burn-up monitor

PIE and separate effect test of high burnup UO2 fuel

International Nuclear Information System (INIS)

Yang, Yong Sik; Kim, S.K.; Kim, D.H.

2005-01-01

To investigate the performance of a high burnup UO 2 fuel, the highest burnup fuel assembly in KOREA was transported to the PIE facility in KAERI. It was a 17·17 fuel assembly irradiated at the Ulchin Unit 2 PWR. The peak fuel rod average burnup was about 57MWd/kgU and locally 65MWd/kgU. The general PIE was performed to investigate the fuel rod irradiation performance. Fission gas release, burnup, oxide thickness, hydrogen pickup, CRUD, and density change were measured by destructive of non-destructive test. Microstructure change, bubble and pore size distributions were observed by optical microscopy, SEM and EPMA. All generated and available PIE results were used to verify high burnup fuel performance code INFRA. Several rods were cut for additional separate effect test. For the high burnup fission gas release behaviour analysis, annealing apparatus were developed and installed in hot cell and preliminary test was performed. In addition to current apparatus new induction furnace will be installed in hot cell to investigate the high temperature and transient fission gas release behaviour. Ring tensile test was performed to analyze the material property degradation which caused by the oxidation and hydride, and additional mechanical tests will be performed. (Author)

Criticality reference benchmark calculations for burnup credit using spent fuel isotopics

International Nuclear Information System (INIS)

Bowman, S.M.

1991-04-01

To date, criticality analyses performed in support of the certification of spent fuel casks in the United States do not take credit for the reactivity reduction that results from burnup. By taking credit for the fuel burnup, commonly referred to as ''burnup credit,'' the fuel loading capacity of these casks can be increased. One of the difficulties in implementing burnup credit in criticality analyses is that there have been no critical experiments performed with spent fuel which can be used for computer code validation. In lieu of that, a reference problem set of fresh fuel critical experiments which model various conditions typical of light water reactor (LWR) transportation and storage casks has been identified and used in the validation of SCALE-4. This report documents the use of this same problem set to perform spent fuel criticality benchmark calculations by replacing the actual fresh fuel isotopics from the experiments with six different sets of calculated spent fuel isotopics. The SCALE-4 modules SAS2H and CSAS4 were used to perform the analyses. These calculations do not model actual critical experiments. The calculated k-effectives are not supposed to equal unity and will vary depending on the initial enrichment and burnup of the calculated spent fuel isotopics. 12 refs., 11 tabs

MOX fuel: a contribution to disarmament. U.S. utilities' response to DOE's plutonium disposition decision

International Nuclear Information System (INIS)

Wallace, M.

1997-01-01

The author is chairman of the Nuclear Energy Institute Plutonium Disposition Working Group, which includes 11 nuclear utilities, including Ontario Hydro, and all the European fabricators of mixed oxide (MOX) fuel. A feasibility study is going on, to see if Russian or other weapons grade plutonium made into MOX fuel can be used in US, Canadian, or other power reactors. The US nuclear power industry is going through a period of change, and its primary responsibility must be the safe, reliable and economic operation of its plants. There is no current US MOX capacity, but the Europeans have have manufactured and burned over 400 tons of MOX fuel since 1963. Canada may be involved, initially through a pilot-scale experiment in NRU reactor

Nuclear Fuel Design Technology Development for the Future Fuel

Energy Technology Data Exchange (ETDEWEB)

Koo, Yang Hyun; Lee, Byung Ho; Cheon, Jin Sik; Oh, Je Yong; Yim, Jeong Sik; Sohn, Dong Seong; Lee, Byung Uk; Ko, Han Suk; So, Dong Sup; Koo, Dae Seo

2006-04-15

The test MOX fuels have been irradiated in the Halden reactor, and their burnup attained 40 GWd/t as of October 2005. The fuel temperature and internal pressure were measured by the sensors installed in the fuels and test rig. The COSMOS code, which was developed by KAERI, well predicted in-reactor behavior of MOX fuel. The COSMOS code was verified by OECD-NEA benchmarks, and the result confirmed the superiority of COSMOS code. MOX in-pile database (IFA-629.3, IFA-610.2 and 4) in Halden was also used for the verification of code. The COSMOS code was improved by introducing Graphic User Interface (GUI) and batch mode. The PCMI analysis module was developed and introduced by the new fission gas behavior model. The irradiation test performed under the arbitrary rod internal pressure could also be analyzed with the COSMOS code. Several presentations were made for the preparation to transfer MOX fuel performance analysis code to the industry, and the transfer of COSMOS code to the industry is being discussed. The user manual and COSMOS program (executive file) were provided for the industry to test the performance of COSMOS code. To envisage the direction of research, the MOX fuel research trend of foreign countries, specially focused on USA's GENP policy, was analyzed.

Models for fuel rod behaviour at high burnup

Energy Technology Data Exchange (ETDEWEB)

Jernkvist, Lars O.; Massih, Ali R. [Quantum Technologies AB, Uppsala Science Park, Uppsala (Sweden)

2004-12-01

This report deals with release of fission product gases and irradiation-induced restructuring in uranium dioxide nuclear fuel. Waterside corrosion of zirconium alloy clad tubes to light water reactor fuel rods is also discussed. Computational models, suitable for implementation in the FRAPCON-3.2 computer code, are proposed for these potentially life-limiting phenomena. Hence, an integrated model for the calculation or thermal fission gas release by intragranular diffusion, gas trapping in grain boundaries, irradiation-induced re-solution, grain boundary saturation, and grain boundary sweeping in UO{sub 2} fuel, under time varying temperature loads, is formulated. After a brief review of the status of thermal fission gas release modelling, we delineate the governing equations for the aforementioned processes. Grain growth kinetic modelling is briefly reviewed and pertinent data on grain growth of high burnup fuel obtained during power ramps in the Third Risoe Fission Gas Release Project are evaluated. Sample computations are performed, which clearly show the connection between fission gas release and gram growth as a function of time at different isotherms. Models are also proposed for the restructuring of uranium dioxide fuel at high burnup, the so-called rim formation, and its effect on fuel porosity build-up, fuel thermal conductivity and fission gas release. These models are assessed by use of recent experimental data from the High Burnup Rim Project, as well as from post irradiation examinations of high-burnup fuel, irradiated in power reactors. Moreover, models for clad oxide growth and hydrogen pickup in PWRs, applicable to Zircaloy-4, ZIRLO or M5 cladding, are formulated, based on recent in-reactor corrosion data for high-burnup fuel rods. Our evaluation of these data indicates that the oxidation rate of ZIRLO-type materials is about 20% lower than for standard Zircaloy-4 cladding under typical PWR conditions. Likewise, the oxidation rate of M5 seems to be

Fabrication, inspection, and test plan for the Advanced Test Reactor (ATR) Mixed-Oxide (MOX) fuel irradiation project

International Nuclear Information System (INIS)

Wachs, G.W.

1997-11-01

The Department of Energy (DOE) Fissile Materials Disposition Materials Disposition Program (FMDP) has announced that reactor irradiation of MOX fuel is one of the preferred alternatives for disposal of surplus weapons-usable plutonium (Pu). MOX fuel has been utilized domestically in test reactors and on an experimental basis in a number of Commercial Light Water Reactors (CLWRs). Most of this experience has been with Pu derived from spent low enriched uranium (LEU) fuel, known as reactor grade (RG) Pu. The MOX fuel test will be irradiated in the ATR to provide preliminary data to demonstrate that the unique properties of surplus weapons-derived or weapons-grade (WG) plutonium (Pu) do not compromise the applicability of this MOX experience base. In addition, the test will contribute experience with irradiation of gallium-containing fuel to the data base required for resolution of generic CLWR fuel design issues (ORNL/MD/LTR-76). This Fabrication, Inspection, and Test Plan (FITP) is a level 2 document as defined in the FMDP LWR MOX Fuel Irradiation Test Project Plan (ORNL/MD/LTR-78)

Determination of enrichment of recycle uranium fuels for different burnup values

International Nuclear Information System (INIS)

Zabunoglu, Okan H.

2008-01-01

Uranium (U) recovered from spent LWR fuels by reprocessing, which contains small amounts of U-236, is to be enriched before being re-irradiated as the recycle U. During the enrichment of recovered U in U-235, the mass fraction of U-236 also increases. Since the existence of U-236 in the recycle U has a negative effect on neutron economy, a greater enrichment of U-235 in the recycle U is required for reaching the same burnup as can be reached by the fresh U fuel. Two burnup values play the most important role in determining the enrichment of recycle U: (1) discharge burnup of spent fuel from which the recycle U is obtained and (2) desired discharge burnup of the recycle U fuel. A step-by-step procedure for calculating the enrichment of the recycle U as a function of these two burnup values is introduced. The computer codes MONTEBURNS and ORIGEN-S are made use of and a three-component (U-235, U-236, U-238) enrichment scheme is applied for calculating the amount of U-236 in producing the recycle U from the recovered U. As was aimed, the resulting expression is simple enough for quick/hand calculations of the enrichment of the recycle U for any given discharge burnup of spent fuel and for any desired discharge burnup of the recycle U fuel, most accurately within the range of 33,000-50,000 MWd/tonU

Burnup performance of rock-like oxide (ROX) fuel in small pebble bed reactor with accumulative fuel loading scheme

International Nuclear Information System (INIS)

Simanullang, Irwan Liapto; Obara, Toru

2017-01-01

Highlights: • Burnup performance using ROX fuel in PBR with accumulative fuel loading scheme was analyzed. • Initial excess reactivity was suppressed by reducing 235 U enrichment in the startup condition. • Negative temperature coefficient was achieved in all condition of PBR with accumulative fuel loading scheme using ROX fuel. • Core lifetime of PBR with accumulative fuel loading scheme using ROX fuel was shorter than with UO 2 fuel. • In PBR with accumulative fuel loading scheme using ROX fuel, achieved discharged burnup can be as high as that for UO 2 fuel. - Abstract: The Japan Atomic Energy Agency (JAEA) has proposed rock-like oxide (ROX) fuel as a new, once-through type fuel concept. Here, burnup performance using ROX fuel was simulated in a pebble bed reactor with an accumulative fuel loading scheme. The MVP-BURN code was used to simulate the burnup calculation. Fuel of 5 g-HM/pebble with 20% 235 U enrichment was selected as the optimum composition. Discharged burnup could reach up to 218 GWd/t, with a core lifetime of about 8.4 years. However, high excess reactivity occurred in the initial condition. Initial fuel enrichment was therefore reduced from 20% to 4.65% to counter the initial excess reactivity. The operation period was reduced by the decrease of initial fuel enrichment, but the maximum discharged burnup was 198 GWd/t. Burnup performance of ROX fuel in this reactor concept was compared with that of UO 2 fuel obtained previously. Discharged burnup for ROX fuel in the PBR with an accumulative fuel loading scheme was as high as UO 2 fuel. Maximum power density could be lowered by introducing ROX fuel compared to UO 2 fuel. However, PBR core lifetime was shorter with ROX fuel than with UO 2 fuel. A negative temperature coefficient was achieved for both UO 2 and ROX fuels throughout the operation period.

Novel technique for manipulating MOX fuel particles using radiation pressure of a laser light

International Nuclear Information System (INIS)

Omori, R.; Suzuki, A.

2001-01-01

We proposed two principles based on the laser manipulation technique for collecting MOX fuel particles floating in air. While Principle A was based on the acceleration of the MOX particles due to the radiation pressure of a visible laser light, Principle B was based on the gradient forces exerted on the particles when an infrared laser light was incident. Principle A was experimentally verified using MnO 2 particles. Numerical results also showed the possibility of collecting MOX fuel particles based on both the principles. (authors)

Discrimination of irradiated MOX fuel from UOX fuel by multivariate statistical analysis of simulated activities of gamma-emitting isotopes

Science.gov (United States)

Åberg Lindell, M.; Andersson, P.; Grape, S.; Hellesen, C.; Håkansson, A.; Thulin, M.

2018-03-01

This paper investigates how concentrations of certain fission products and their related gamma-ray emissions can be used to discriminate between uranium oxide (UOX) and mixed oxide (MOX) type fuel. Discrimination of irradiated MOX fuel from irradiated UOX fuel is important in nuclear facilities and for transport of nuclear fuel, for purposes of both criticality safety and nuclear safeguards. Although facility operators keep records on the identity and properties of each fuel, tools for nuclear safeguards inspectors that enable independent verification of the fuel are critical in the recovery of continuity of knowledge, should it be lost. A discrimination methodology for classification of UOX and MOX fuel, based on passive gamma-ray spectroscopy data and multivariate analysis methods, is presented. Nuclear fuels and their gamma-ray emissions were simulated in the Monte Carlo code Serpent, and the resulting data was used as input to train seven different multivariate classification techniques. The trained classifiers were subsequently implemented and evaluated with respect to their capabilities to correctly predict the classes of unknown fuel items. The best results concerning successful discrimination of UOX and MOX-fuel were acquired when using non-linear classification techniques, such as the k nearest neighbors method and the Gaussian kernel support vector machine. For fuel with cooling times up to 20 years, when it is considered that gamma-rays from the isotope 134Cs can still be efficiently measured, success rates of 100% were obtained. A sensitivity analysis indicated that these methods were also robust.

Simulation of integral local tests with high-burnup fuel

International Nuclear Information System (INIS)

Gyori, G.

2011-01-01

The behaviour of nuclear fuel under LOCA conditions may strongly depend on the burnup-dependent fuel characteristics, as it has been indicated by recent integral experiments. Fuel fragmentation and the associated fission gas release can influence the integral fuel behaviour, the rod rupture and the radiological release. The TRANSURANUS fuel performance code is a proper tool for the consistent simulation of burnup-dependent phenomena during normal operation and the thermo-mechanical behaviour of the fuel rod in a subsequent accident. The code has been extended with an empirical model for micro-cracking induced FGR and fuel fragmentation and verified against integral LOCA tests of international projects. (author)

Sodium fast reactor: an asset for a PWR UOX/MOX fleet - 5327

International Nuclear Information System (INIS)

Tiphine, M.; Coquelet-Pascal, C.; Girieud, R.; Eschbach, R.; Chabert, C.; Grosman, R.

2015-01-01

Due to its low fissile content, Pu from spent MOX fuels is sometimes regarded as not recyclable in LWR. Based on the existing French nuclear infrastructure (La Hague reprocessing plant and MELOX MOX manufacturing plant), AREVA and CEA have evaluated the conditions of Pu multi recycling in a 100% LWR fleet. As France is currently supporting a Fast Reactor prototype project, scenario studies have also been conducted to evaluate the contribution of a 600 MWe SFR in the LWR fleet. These scenario studies consider a nuclear fleet composed of 8 PWR 900 MWe, with or without the contribution of a SFR, and aim at evaluating the following points: -) the feasibility of Pu multi-recycling in PWR; -) the impact on the spent fuels storage; -) the reduction of the stored separated Pu; -) the impact on waste management and final disposal. The studies have been conducted with the COSI6 code, developed by CEA Nuclear Energy Direction since 1985, that simulates the evolution over time of a nuclear power plants fleet and of its associated fuel cycle facilities and provides material flux and isotopic compositions at each point of the scenario. To multi-recycle Pu into LWR MOX and to ensure flexibility, different reprocessing strategies were evaluated by adjusting the reprocessing order, the choice of used fuel assemblies according to their burn-up and the UOX/MOX proportions. The improvement of the Pu fissile quality and the kinetic of Pu multi-recycling in SFR depending on the initial Pu quality were also evaluated and led to a reintroduction of Pu in PWR MOX after a single irradiation in SFR, still in dilution with Pu from UOX to maintain a sufficient fissile quality. (authors)

Impact of extended burnup on the nuclear fuel cycle

International Nuclear Information System (INIS)

1993-04-01

The Advisory Group Meeting was held in Vienna from 2 to 5 December 1991, to review, analyse, and discuss the effects of burnup extension in both light and heavy water reactors on all aspects of the fuel cycle. Twenty experts from thirteen countries participated in this meeting. There was consensus that both economic and environmental benefits are driving forces toward the achievement of higher burnups and that the present trend of burnup extension may be expected to continue. The extended burnup has been considered for the three main stages of the fuel cycle: the front end, in-reactor issues and the back end. Thirteen papers were presented. A separate abstract was prepared for each of these papers. Refs, figs and tabs

Application of burnup credit in spent fuel management at Russian NPPs

International Nuclear Information System (INIS)

Koulikov, V.I.; Makarchuk, T.F.; Tikhonov, N.S.

1998-01-01

The article concerns implementation of burnup credit in spent fuel storage and transportation. Some of the problems with increased enrichment fuel can be resolved by use of modified transport methodology. Such as shipping in gas-filled casks only, reduced number of assemblies in casks, etc. However, the use of modified schemes of transportation results in essential financial losses. An actinide-only burnup credit is taken into account in most part of criticality calculations, and a parameter limiting loading of spent fuel in the cask or the repository is the avenge value of burnup on an assembly. The main method of burnup depth definition is its defect measurement. A short description of devices for measurement as well as some technical results of suing burnup credit approach in storage and transport are given. (author)

ORIGEN-2 libraries based on JENDL-3.2 for PWR-MOX fuel

Energy Technology Data Exchange (ETDEWEB)

Matsumoto, Hideki; Onoue, Masaaki; Tahara, Yoshihisa [Mitsubishi Heavy Industries Ltd., Tokyo (Japan)

2001-08-01

A set of ORIGEN-2 libraries for PWR MOX fuel was developed based on JENDL-3.2 in the Working Group on Evaluation of Nuclide Production, Japanese Nuclear Data Committee. The calculational model generating ORIGEN-2 libraries of PWR MOX is explained here in detail. The ORIGEN-2 calculation with the new ORIGEN-2 MOX library can predict the nuclides contents within 10% for U and Pu isotopes and 20% for both minor actinides and main FPs. (author)

Main trends and content of works on fabrication of fuel rods with MOX fuel for the WWER-1000 reactor

International Nuclear Information System (INIS)

Tsykanov, V.A.; Golovanov, V.N.; Mayorshin, A.A.; Yurchenko, A.D.; Ilyenko, S.A.; Syuzev, V.N.

2000-01-01

The main trends of production of pellet MOX-fuel for the WWER reactors using the trial-experimental equipment at SSC RF RIAR are set forth. The main realized parameters of fabrication of MOX-fuel pellets are presented. The content of the reactor tests program is considered with allowance for their licensing requirements for the WWER reactors. (author)

Modelling of some high burnup phenomena in nuclear fuel

Energy Technology Data Exchange (ETDEWEB)

Forsberg, K; Lindstroem, F; Massih, A R [ABB Atom AB, Vaesteraas (Sweden)

1997-08-01

In this paper the results of some modelling efforts carried out by ABB Atom to describe certain light water reactor fuel high burnup effects are presented. In particular the degradation of fuel thermal conductivity with burnup and its impact on fuel temperature is briefly discussed. The formation of a porous rim and its effect on a thermal fission gas release has been modelled and the model has been used to predict the release of pressurized water reactor fuel rods that were operated at low power densities. Furthermore, a mathematical model which combines the diffusion and re-solution controlled thermal release with grain boundary movement has been briefly described. The model is used to compare release with diffusion only and release caused by diffusion and grain boundary sweeping (due to grain growth). Finally, analytical expressions are obtained for the calculation of fuel stoichiometry as a function of burnup. (author). 20 refs, 10 figs, 1 tab.

Progress of full MOX core design in ABWR

International Nuclear Information System (INIS)

Izutsu, S.; Sasagawa, M.; Aoyama, M.; Maruyama, H.; Suzuki, T.

2000-01-01

Full MOX ABWR core design has been made, based on the MOX design concept of 8x8 bundle configuration with a large central water rod, 40 GWd/t maximum bundle exposure, and the compatibility with 9x9 high-burnup UO 2 bundles. Core performance on shutdown margin and thermal margin of the MOX-loaded core is similar to that of UO 2 cores for the range from full UO 2 core to full MOX core. Safety analyses based on its safety parameters and MOX property have shown its conformity to the design criteria in Japan. In order to confirm the applicability of the nuclear design method to full MOX cores, Tank-type Critical Assembly (TCA) experiment data have been analyzed on criticality, power distribution and β eff /l measurements. (author)

Study on transport safety of fresh MOX fuel. Performance of the cladding tube of fresh MOX fuel against external water pressure

International Nuclear Information System (INIS)

Ito, Chihiro

1999-01-01

It is important to know the ability of the cladding tube for fresh MOX fuel against external water pressure when they were hypothetically sunk into the sea for unknown reasons. In order to evaluate the ability of cladding tubes for MOX fresh fuel against external water pressure, external water pressure tests were carried out. Resistible limit of cladding tubes against external water pressure is defined when cladding tubes are deformed largely due to buckling etc. The test results show cladding tube of BWR type can resist an external water pressure of 69 MPa (a depth of water of 7,000 m) and that of PWR type fuel can resist an external water pressure of 54 MPa (a depth of water of 5,500 m). Moreover, leak tightness is maintained at an external water pressure of 73 MPa (a depth of water of 7,400 m) for BWR type cladding tubes and at an external water pressure of 98 MPa (a depth of water of 10,000 m) for PWR type cladding tubes. (author)

Image analysis: a tool characterising and modelling the microstructure of the MOX fuel

International Nuclear Information System (INIS)

Charollais, F.

1997-01-01

The MOX nuclear fuel, made up of about 3 to 10 % of plutonium oxide mixed with uranium oxide, is elaborated by an original manufacturing method (MIMAS process). The MOX pellets feature a singular and complex microstructure, including enriched plutonium zones dispersed in a low plutonium content matrix. Their properties as well as their performances levels are strongly linked with this microstructure. Tools, found in the literature, allowing to quantify with relevant parameters the microstructural images from different analytical equipment (optical microscopy, electron probe micro-analyser and autoradiography) have been adapted and used in order to characterize these nuclear fuels. Taking into account the heterogeneity of the MOX microstructure, we turn our's attention, at the beginning of this study, to the analysis conditions: choice of the magnification, sampling and statistical analysis of the measurements. An improvement of the ceramographic preparation of the samples, required for an automatic image analysis (of the granular structure), has been realised by thermal etching under oxidizing gas. This method enables the strong content plutonium zones to be revealed distinctly. The first part of the study concerns the characterization of the three-dimensional structure of uranium oxide and MOX fuels by average variables using the principles of mathematical morphology and stereology. The second part introduces probabilistic models, in particular the Boolean scheme, in order to improve and complete the three-dimensional characterization of the MOX fuel and more specifically the enriched plutonium islands dispersion in the pellet. [fr

Estimate of the Sources of Plutonium-Containing Wastes Generated from MOX Fuel Production in Russia

International Nuclear Information System (INIS)

Kudinov, K. G.; Tretyakov, A. A.; Sorokin, Yu. P.; Bondin, V. V.; Manakova, L. F.; Jardine, L. J.

2002-01-01

In Russia, mixed oxide (MOX) fuel is produced in a pilot facility ''Paket'' at ''MAYAK'' Production Association. The Mining-Chemical Combine (MCC) has developed plans to design and build a dedicated industrial-scale plant to produce MOX fuel and fuel assemblies (FA) for VVER-1000 water reactors and the BN-600 fast-breeder reactor, which is pending an official Russian Federation (RF) site-selection decision. The design output of the plant is based on a production capacity of 2.75 tons of weapons plutonium per year to produce the resulting fuel assemblies: 1.25 tons for the BN-600 reactor FAs and the remaining 1.5 tons for VVER-1000 FAs. It is likely the quantity of BN-600 FAs will be reduced in actual practice. The process of nuclear disarmament frees a significant amount of weapons plutonium for other uses, which, if unutilized, represents a constant general threat. In France, Great Britain, Belgium, Russia, and Japan, reactor-grade plutonium is used in MOX-fuel production. Making MOX-fuel for CANDU (Canada) and pressurized water reactors (PWR) (Europe) is under consideration in Russia. If this latter production is added, as many as 5 tons of Pu per year might be processed into new FAs in Russia. Many years of work and experience are represented in the estimates of MOX fuel production wastes derived in this report. Prior engineering studies and sludge treatment investigations and comparisons have determined how best to treat Pu sludges and MOX fuel wastes. Based upon analyses of the production processes established by these efforts, we can estimate that there will be approximately 1200 kg of residual wastes subject to immobilization per MT of plutonium processed, of which approximately 6 to 7 kg is Pu in the residuals per MT of Pu processed. The wastes are various and complicated in composition. Because organic wastes constitute both the major portion of total waste and of the Pu to be immobilized, the recommended treatment of MOX-fuel production waste is

Estimate of the Sources of Plutonium-Containing Wastes Generated from MOX Fuel Production in Russia

Energy Technology Data Exchange (ETDEWEB)

Kudinov, K. G.; Tretyakov, A. A.; Sorokin, Yu. P.; Bondin, V. V.; Manakova, L. F.; Jardine, L. J.

2002-02-26

In Russia, mixed oxide (MOX) fuel is produced in a pilot facility ''Paket'' at ''MAYAK'' Production Association. The Mining-Chemical Combine (MCC) has developed plans to design and build a dedicated industrial-scale plant to produce MOX fuel and fuel assemblies (FA) for VVER-1000 water reactors and the BN-600 fast-breeder reactor, which is pending an official Russian Federation (RF) site-selection decision. The design output of the plant is based on a production capacity of 2.75 tons of weapons plutonium per year to produce the resulting fuel assemblies: 1.25 tons for the BN-600 reactor FAs and the remaining 1.5 tons for VVER-1000 FAs. It is likely the quantity of BN-600 FAs will be reduced in actual practice. The process of nuclear disarmament frees a significant amount of weapons plutonium for other uses, which, if unutilized, represents a constant general threat. In France, Great Britain, Belgium, Russia, and Japan, reactor-grade plutonium is used in MOX-fuel production. Making MOX-fuel for CANDU (Canada) and pressurized water reactors (PWR) (Europe) is under consideration in Russia. If this latter production is added, as many as 5 tons of Pu per year might be processed into new FAs in Russia. Many years of work and experience are represented in the estimates of MOX fuel production wastes derived in this report. Prior engineering studies and sludge treatment investigations and comparisons have determined how best to treat Pu sludges and MOX fuel wastes. Based upon analyses of the production processes established by these efforts, we can estimate that there will be approximately 1200 kg of residual wastes subject to immobilization per MT of plutonium processed, of which approximately 6 to 7 kg is Pu in the residuals per MT of Pu processed. The wastes are various and complicated in composition. Because organic wastes constitute both the major portion of total waste and of the Pu to be immobilized, the recommended treatment

Technical design considerations in the provision of a commercial MOX plant

International Nuclear Information System (INIS)

Elliott, M.F.

1997-01-01

The Sellafield MOX Plant (SMP) has a design production target of 120 t/year Heavy Metal of mixed uranium dioxide and plutonium dioxided (MOX) fuel. It will have the capability to produce fuel with fissile enrichments up to 10%. The feed materials are those arising from reprocessing operations on the Sellafield site, although the plant also has the capability to receive and process plutonium from overseas reprocessing plants. The ability to produce 10% enriched fuels, together with the requirement to use high burn-up feed has posed a number of design challenges to prevent excessive powder temperatures within the plant. As no stimulants are available to represent the heat generating nature of plutonium powders, it is difficult to prove equipment design by experiment. Extensive use has therefore been made of finite element analysis techniques. The requirement to process material of low burn-up (i.e. high fissile enrichment) has also impacted on equipment design in order to ensure that criticality limits are not exceeded. This has been achieved where possible by 'safe by geometry' design and, where appropriate, by high integrity protection systems. SMP has been designed with a high plant availability but at minimum cost. The requirement to minimize cost has meant that high availability must be obtained with the minimum of equipment. This had led to major challenges for equipment designers in terms of both the reliability and also the maintainability of equipment. Extensive use has been made of theoretical modelling techniques which have given confidence that plant throughput can be achieved. (author). 1 fig

Fission gas release from fuels at high burnup

International Nuclear Information System (INIS)

Kauffmann, Yves; Pointud, M.L.; Vignesoult, Nicole; Atabek, Rosemarie; Baron, Daniel.

1982-04-01

Determinations of residual gas concentrations by heating and by X microanalysis were respectively carried out on particles (TANGO program) and on sections of fuel rods, perfectly characterized as to fabrication and irradiation history. A threshold release temperature of 1250 0 C+-100 0 C was determined irrespective of the type of oxide and the irradiation history in the 18,000-45,000 MWdt -1 (U) specific burnup field. The overall analyses of gas released from the fuel rods show that, in the PWR operating conditions, the fraction released remains less than 1% up to a mean specific burnup of 35000 MWdt -1 (U). The release of gases should not be a limiting factor in the increase of specific burnups [fr

Argentine nuclear fuels MOX irradiated in the Petten reactor: Analysis of experience with the BACO code

Energy Technology Data Exchange (ETDEWEB)

Marino, A C; Perez, E; Adelfang, P [Argentine Atomic Energy Commission, Buenos Aires (Argentina)

1997-08-01

The irradiation of our first prototypes of MOX nuclear fuels fabricated in Argentina began in 1986. These experiences had been made in the HFR-Petten reactor, Holland. The six rods were fabricated in the {alpha} Facility (GAID-CNEA-Argentina). The first rod has been used for destructive pre-irradiation analysis in the KFK (Kernforschungszentrum Karlsruhe), Germany. The second one was a pathfinder for calibrating systems in the HFR. Another two rods included doped pellets based on iodine. One of them included CsI and auxiliary components. The second one included elemental iodine. The concentration of iodine was intended to simulate 15 MWd/ton(M) of burnup. We defined the power histories with the BACO code. We assumed a cycle of 15 days that included interaction treatments of cladding and pellet due to the power cycling. The last ramp is let run until stress corrosion cracking (SCC) is induced. The experience named BU15 was done with the last two rods. The final burnup was 15 MWd/ton(M), and a final ramp test was arranged for one of them. This burnup is the same as the previous two rods. The power level during irradiation was low and without major solicitations, only the normal shutdowns of the HFR. The ramp was similar to that used for the iodine test. We attempt to see the correct correspondence between the BU15 and the doping test. The pathfinder had an excellent behavior in the HFR reactor. The presence of microcracks inside the cladding was observed in the iodine test as we predicted with the BACO code. The post-irradiation tests of the BU15 experience has just ended. The development of the ramp was interrupted due to an increase of activity in the system. We presumed the presence of a failure in the rod. The visual inspection of the rod shows an atypical failure for this kind of fuel, i.e. they found a small circular hole. We use the BACO code for the behavior analysis of the fuel rods. 23 refs, 29 figs, 5 tabs.

Argentine nuclear fuels MOX irradiated in the Petten reactor: Analysis of experience with the BACO code

International Nuclear Information System (INIS)

Marino, A.C.; Perez, E.; Adelfang, P.

1997-01-01

The irradiation of our first prototypes of MOX nuclear fuels fabricated in Argentina began in 1986. These experiences had been made in the HFR-Petten reactor, Holland. The six rods were fabricated in the α Facility (GAID-CNEA-Argentina). The first rod has been used for destructive pre-irradiation analysis in the KFK (Kernforschungszentrum Karlsruhe), Germany. The second one was a pathfinder for calibrating systems in the HFR. Another two rods included doped pellets based on iodine. One of them included CsI and auxiliary components. The second one included elemental iodine. The concentration of iodine was intended to simulate 15 MWd/ton(M) of burnup. We defined the power histories with the BACO code. We assumed a cycle of 15 days that included interaction treatments of cladding and pellet due to the power cycling. The last ramp is let run until stress corrosion cracking (SCC) is induced. The experience named BU15 was done with the last two rods. The final burnup was 15 MWd/ton(M), and a final ramp test was arranged for one of them. This burnup is the same as the previous two rods. The power level during irradiation was low and without major solicitations, only the normal shutdowns of the HFR. The ramp was similar to that used for the iodine test. We attempt to see the correct correspondence between the BU15 and the doping test. The pathfinder had an excellent behavior in the HFR reactor. The presence of microcracks inside the cladding was observed in the iodine test as we predicted with the BACO code. The post-irradiation tests of the BU15 experience has just ended. The development of the ramp was interrupted due to an increase of activity in the system. We presumed the presence of a failure in the rod. The visual inspection of the rod shows an atypical failure for this kind of fuel, i.e. they found a small circular hole. We use the BACO code for the behavior analysis of the fuel rods. 23 refs, 29 figs, 5 tabs

Estimate of the Sources of Plutonium-Containing Wastes Generated from MOX Fuel Production in Russia

International Nuclear Information System (INIS)

Kudinov, K.G.; Tretyakov, A.A.; Sorokin, Y.P.; Bondin, V.V.; Manakova, L.F.; Jardine, L.J.

2001-01-01

In Russia, mixed oxide (MOX) fuel is produced in a pilot facility ''Paket'' at ''MAYAK'' Production Association. The Mining-Chemical Combine (MCC) has developed plans to design and build a dedicated industrial-scale plant to produce MOX fuel and fuel assemblies (FA) for VVER-1000 water reactors and the BN-600 fast-breeder reactor, which is pending an official Russian Federation (RF) site-selection decision. The design output of the plant is based on production capacity of 2.75 tons of weapons plutonium per year to produce the resulting fuel assemblies: 1.25 tons for the BN-600 reactor FAs and the remaining 1.5 tons for VVER-1000 FAs. It is likely the quantity of BN-600 FAs will be reduced in actual practice. The process of nuclear disarmament frees a significant amount of weapons plutonium for other uses, which, if unutilized, represents a constant general threat. In France, Great Britain, Belgium, Russia, and Japan, reactor-grade plutonium is used in MOX-fuel production. Making MOX-fuel for CANDU (Canada) and pressurized water reactors (PWR) (Europe) is under consideration Russia. If this latter production is added, as many as 5 tons of Pu per year might be processed into new FAs in Russia. Many years of work and experience are represented in the estimates of MOX fuel production wastes derived in this report. Prior engineering studies and sludge treatment investigations and comparisons have determined how best to treat Pu sludges and MOX fuel wastes. Based upon analyses of the production processes established by these efforts, we can estimate that there will be approximately 1200 kg of residual wastes subject to immobilization per MT of plutonium processed, of which approximately 6 to 7 kg is Pu in the residuals per MT of Pu processed. The wastes are various and complicated in composition. Because organic wastes constitute both the major portion of total waste and of the Pu to be immobilized, the recommended treatment of MOX-fuel production waste is incineration

Calculation of fuel burn-up and fuel reloading for the Dalat Nuclear Research Reactor

Energy Technology Data Exchange (ETDEWEB)

Lan, Nguyen Phuoc; Huy, Ngo Quang [Centre for Nuclear Technique Application, Ho Chi Minh City (Viet Nam); Thong, Ha Van; Binh, Do Quang [Nuclear Research Inst., Da Lat (Viet Nam)

1994-10-01

Calculation of fuel burnup and fuel reloading for the Dalat Nuclear Research Reactor was carried out by using a new programme named HEXA-BURNUP, realized in a PC. The programme is used to calculate the following parameters of the Dalat reactor: a/Critical configurations of the core loaded with 69, 72, 74, 86, 88, 89 and 92 fuel elements. The effective multiplication coefficients equal 1 within the error ranges of less than 0.38%. b/ The thermal neutron flux distribution in the reactor. The calculated results agree with the experimental data measured at 11 typical positions. c/The average fuel burn-up for the period from Feb. 1984 to Sep. 1992. The difference between calculation and experiment is only about 1.9%. 10 fuel reloading versions are calculated, from which an optimal version is proposed. (author). 9 refs., 4 figs., 5 tabs.

Revised conceptual designs for the FMDP MOX fresh fuel transport package

International Nuclear Information System (INIS)

Ludwig, S.B.; Michelhaugh, R.D.; Shappert, L.B.; Chae, S.M.; Tang, J.S.

1998-03-01

The revised conceptual designs described in this document provide a foundation for the development and certification of final transport package designs that will be needed to support the disposition of surplus weapons-grade plutonium as mixed-oxide (MOX) fuel in commercial light-water reactors in the US. This document is intended to describe the revised package design concepts and summarize the results of preliminary analyses and assessments of two new concepts for fresh MOX fuel transport packages that have been developed by Oak Ridge National Laboratory during the past year in support of the Department of Energy/Office of Fissile Materials Disposition

In-core fuel management and perspectives

International Nuclear Information System (INIS)

Waeckel, N.

2009-01-01

The management of nuclear fuel inside the core has to take into account the necessity to stop the reactor periodically to renew the fuel partially and to perform maintenance operations. The fuel management strategy determines the cost of the fuel (through the number of assemblies that have been changed and their enrichment rate) and the duration of the campaign till next stop. Fuel management strategies have to conciliate different objectives: -) the safety of the reactor, -) the reliability of the fuel assemblies, -) the optimization of the fuel cost by increasing the discharge burnup. The necessity of spent fuel processing implies a maximal discharge burnup. During the 1990-2000 period, the discharge burnups have been progressively increased through the following fuel management strategies: Garance, Cyclades and Gemmes. During the years 2000-2009, the progressive absorption of the nuclear over-equipment, the opening of the European electricity markets favored power production through the MOX-parity, Alcade and Galice fuel management strategies. The perspective for next decade is to favor production to the prejudice of higher burnups. (A.C.)

Method for adding additional isotopes to actinide-only burnup credit

International Nuclear Information System (INIS)

Lancaster, D.B.; Fuentes, E.; Kang, C.

1998-01-01

The Topical Report on Actinide-Only Burnup Credit for Pressurized Water Reactor Spent Nuclear Fuel Packages requires computer code validation to be performed against a benchmark set of chemical assays for isotopic concentration and against a benchmark set of critical experiments for package criticality. Both sets contain all the isotopes included in the methodology. The chemical assays used include the uranium and plutonium isotopes, while the critical experiments were composed of UO 2 or MOX rods, covering the isotopes in the actinide only approach. Since other isotopes are not included in the validation benchmark sets, it would be necessary to justify both the content and worth of any additional isotope for which burnup credit is to be taken (i.e., both the concentration and criticality effect of each particular isotope must be validated). A method is proposed here that can be used for any number of additional isotopes. As does the actinide-only burnup credit methodology, this method makes use of chemical assay data to establish the conservatism in the prediction of each isotope's concentration. Criticality validation is also performed using a benchmark set of UO 2 and MOX critical experiments, where the additional isotopes are validated using worth experiments to conservatively account for any uncertainty in their cross sections. The remaining requirements (analysis and modeling parameters, loading criteria generation, and physical implementation and controls) are performed exactly as described in the actinide-only burnup credit methodology. This report provides insight into each particular requirement in the new methodology

Development of MOX manufacturing technology in BNFL

International Nuclear Information System (INIS)

Buchan, P.G.; Powell, D.J.; Edwards, J.

1998-01-01

BNFL is successfully operating a small scale MOX fuel fabrication facility at its Sellafield Site and is currently constructing an advanced, commercial scale MOX facility to complement its existing LWR UO 2 fabrication capability. BNFL's MOX fuel capability is fully supported by a comprehensive technology development programme aimed at providing a high quality product which is successfully competing in the market. Building on the experience gained over the last 30 years, is from the production of both thermal and fast reactor MOX fuels, BNFL's development team set a standard for its MOX product which is targeted at exceeding the performance of UO 2 fuel in reactor. In order to meet the stringent design requirements the product development team has introduced the Short Binderless Route (SBR) process that is now used routinely in BNFL's MOX Demonstration Facility (MDF) and which forms the basis for BNFL's large scale Sellafield MOX Plant. This plant not only uses the SBR process for MOX production but also incorporates the most advanced technology available anywhere in the world for nuclear fuel production. A detailed account of the technology developed by BNFL to support its MOX fuels business will be provided, together with an explanation of the processes and plants used for MOX fuel production by BNFL. The paper also looks at the future needs of the MOX business and how improvements in pellet design can assist the MOX fabrication production process to meet the user demand requirements of utilities around the world. (author)

Nuclear fuel burn-up economy; Ekonomija izgaranja nuklearnog goriva

Energy Technology Data Exchange (ETDEWEB)

Matausek, M [Institute of nuclear sciences Boris Kidric, Vinca, Beograd (Yugoslavia)

1984-07-01

In the period 1981-1985, for the needs of Utility Organization, Beograd, and with the support of the Scientific Council of SR Srbija, work has been performed on the study entitled 'Nuclear Fuel Burn-up Economy'. The forst [phase, completed during the year 1983 comprised: comparative analysis of commercial NPP from the standpoint of nuclear fuel requirements; development of methods for fuel burn-up analysis; specification of elements concerning the nuclear fuel for the tender documentation. The present paper gives the short description of the purpose, content and results achieved in the up-to-now work on the study. (author)

Fission gas release and fuel rod chemistry related to extended burnup

International Nuclear Information System (INIS)

1993-04-01

The purpose of the meeting was to review the state of the art in fission gas release and fuel rod chemistry related to extended burnup. The meeting was held in a time when national and international programmes on water reactor fuel irradiated in experimental reactors were still ongoing or had reached their conclusion, and when lead test assemblies had reached high burnup in power reactors and been examined. At the same time, several out-of-pile experiments on high burnup fuel or with simulated fuel were being carried out. As a result, significant progress has been registered since the last meeting, particularly in the evaluation of fuel temperature, the degradation of the global thermal conductivity with burnup and in the understanding of the impact on fission gas release. Fifty five participants from 16 countries and one international organization attended the meeting. 28 papers were presented. A separate abstract was prepared for each of the papers. Refs, figs, tabs and photos

Plutonium isotopic composition of high burnup spent fuel discharged from light water reactors

International Nuclear Information System (INIS)

Nakano, Yoshihiro; Okubo, Tsutomu

2011-01-01

Highlights: → Pu isotopic composition of fuel affects FBR core nuclear characteristics very much. → Spent fuel compositions of next generation LWRs with burnup of 70 GWd/t were obtained. → Pu isotopic composition and amount in the spent fuel with 70 GWd/t were evaluated. → Spectral shift rods of high burnup BWR increases the fissile Pu fraction of spent fuel. → Wide fuel rod pitch of high burnup PWR lowers the fissile Pu fraction of spent fuel. - Abstract: The isotopic composition and amount of plutonium (Pu) in spent fuel from a high burnup boiling water reactor (HB-BWR) and a high burnup pressurized water reactor (HB-PWR), each with an average discharge burnup of 70 GWd/t, were estimated, in order to evaluate fast breeder reactor (FBR) fuel composition in the transition period from LWRs to FBRs. The HB-BWR employs spectral shift rods and the neutron spectrum is shifted through the operation cycle. The weight fraction of fissile plutonium (Puf) isotopes to the total plutonium in HB-BWR spent fuel after 5 years cooling is 62%, which is larger than that of conventional BWRs with average burnup of 45 GWd/t, because of the spectral shift operation. The amount of Pu produced in the HB-BWR is also larger than that produced in a conventional BWR. The HB-PWR uses a wider pitch 17 x 17 fuel rod assembly to optimize neutron slowing down. The Puf fraction of HB-PWR spent fuel after 5 years cooling is 56%, which is smaller than that of conventional PWRs with average burnup of 49 GWd/t, mainly because of the wider pitch. The amount of Pu produced in the HB-PWR is also smaller than that in conventional PWRs.

Thermal and in-pile densification of MOX fuels: Some recent results

International Nuclear Information System (INIS)

Caillot, L.; Malgouyres, P.P.; Souchon, F.; Gotta, M.J.; Warin, D.; Chotard, A.; Couty, J.C.

1997-01-01

In-pile densification of PWR fuels is one of the main phenomena which determine the evolution of the pellet-clad gap during the first stage of the irradiation, and thus has consequences onto the thermo-mechanical behaviours of fuel rods. It can be predicted using the results of resintering tests and appropriate correlations. In this context, CEA, FRAMATOME and EDF have undertaken a joint research programme aiming to characterize the densification of MOX fuels. Different fuels were prepared by the MIMAS process using different UO 2 powders as matrix. After a detailed characterization, fuel pellets were submitted to isothermal resintering tests and analytical irradiations. Correlations between in-pile and thermal densification were established. This paper presents the results obtained with two types of MOX fuel: one fabricated wit the AUC UO 2 powder (ammonium uranyl carbonate conversion process) and another one fabricated with the SFEROX powder (peroxide conversion process). 8 refs, 8 figs

Design of full MOX core in ABWR

International Nuclear Information System (INIS)

Kinoshita, Y.; Hirose, T.; Sasagawa, M.; Sakuma, T

1999-01-01

A Full MOX-ABWR, loaded with mixed-oxide (MOX) fuels of up to 100% of the core, is planned. Increased MOX fuel utilization will result in greater savings of uranium. Studies on the fuel rod thermal-mechanical design, the core design and the safety evaluation have been made, and the results are summarized in this paper. To sum it all up, the safety of the Full MOX-ABWR has been confirmed through design evaluations adequately considering the MOX fuel and core characteristics. (author)

Continuous process of powder production for MOX fuel fabrication according to ''granat'' technology

International Nuclear Information System (INIS)

Morkovnikov, V.E.; Raginskiy, L.S.; Pavlinov, A.P.; Chernov, V.A.; Revyakin, V.V.; Varykhanov, V.S.; Revnov, V.N.

2000-01-01

During last years the problem of commercial MOX fuel fabrication for nuclear reactors in Russia was solved in a number of directions. The paper deals with the solution of the problem of creating a continuous pilot plant for the production of MOX fuel powders on the basis of the home technology 'Granat', that was tested before on a small-scale pilot-commercial batch-operated plant of the same name and confirmed good results. (authors)

Assessment of US NRC fuel rod behavior codes to extended burnup

International Nuclear Information System (INIS)

Laats, E.T.; Croucher, D.W.; Haggag, F.M.

1982-01-01

The purpose of this paper is to report the status of assessing the capabilities of the NRC fuel rod performance codes for calculating extended burnup rod behavior. As part of this effort, a large spectrum of fuel rod behavior phenomena was examined, and the phenomena deemed as being influential during extended burnup operation were identified. Then, the experiment data base addressing these identified phenomena was examined for availability and completeness at extended burnups. Calculational capabilities of the NRC's steady state FRAPCON-2 and transient FRAP-T6 fuel rod behavior codes were examined for each of the identified phenomenon. Parameters calculated by the codes were compared with the available data base, and judgments were made regarding model performance. Overall, the FRAPCON-2 code was found to be moderately well assessed to extended burnups, but the FRAP-T6 code cannot be adequately assessed until more transient high burnup data are available

Modeling of WWER-440 Fuel Pin Behavior at Extended Burn-up

International Nuclear Information System (INIS)

El-Koliel, M.S.; Abou-Zaid, A.A.; El-Kafas, A.A.

2004-01-01

Currently, there is an ongoing effort to increase fuel discharge burn-up of all LWRs fuel including WWER's as much as possible in order to decrease power production cost. Therefore, burn-up is expected to be increased to 60 to 70 Mwd/kg U. The change in the fuel radial power distribution as a function of fuel burn up can affect the radial fuel temperature distribution as well as the fuel microstructure in the fuel pellet rim. In this paper, the radial burn-up and fissile products distributions of WWER-440 UO 2 fuel pin were evaluated using MCNP 4B and ORIGEN2 codes. The impact of the thermal conductivity on predicted fission gas release calculations is needed. For the analysis, a typical WWER-440 fuel pin and surrounding water moderator are considered in a hexagonal pin cell well. The thermal release and the athermal release from the pellet rim were modeled separately. The fraction of the rim structure and the excessive porosity in the rim structure in isothermal irradiation as a function of the fuel burn-up was predicted. a computer program; RIMSC-01, is developed to perform the required FGR calculations. Finally, the relevant phenomena and the corresponding models together with their validation are presented

ABB PWR fuel design for high burnup

International Nuclear Information System (INIS)

Nilsson, S.; Jourdain, P.; Limback, M.; Garde, A.M.

1998-01-01

Corrosion, hydriding and irradiation induced growth of a based materials are important factors for the high burnup performance of PWR fuel. ABB has developed a number of Zr based alloys to meet the need for fuel that enables operation to elevated burnups. The materials include composition and processing optimised Zircaloy 4 (OPTIN TM ) and Zircaloy 2 (Zircaloy 2P), as well as advanced Zr based alloys with chemical compositions outside the composition specified for Zircaloy. The advanced alloys are either used as Duplex or as single component claddings. The Duplex claddings have an inner component of Zircaloy and an outer layer of Zr with small additions of alloying elements. ABB has furthermore improved the dimensional stability of the fuel assembly by developing stiffer and more bow resistant guide tubes while debris related fuel failures have been eliminated from ABB fuel by introducing the Guardian TM grid. Intermediate flow mixers that improve the thermal hydraulic performance and the dimensional stability of the fuel has also been developed within ABB. (author)

Reactivity effect of spent fuel depending on burn-up history

International Nuclear Information System (INIS)

Hayashi, Takafumi; Suyama, Kenya; Nomura, Yasushi

2001-06-01

It is well known that a composition of spent fuel depends on various parameter changes throughout a burn-up period. In this study we aimed at the boron concentration and its change, the coolant temperature and its spatial distribution, the specific power, the operation mode, and the duration of inspection, because the effects due to these parameters have not been analyzed in detail. The composition changes of spent fuel were calculated by using the burn-up code SWAT, when the parameters mentioned above varied in the range of actual variations. Moreover, to estimate the reactivity effect caused by the composition changes, the criticality calculations for an infinite array of spent fuel were carried out with computer codes SRAC95 or MVP. In this report the reactivity effects were arranged from the viewpoint of what parameters gave more positive reactivity effect. The results obtained through this study are useful to choose the burn-up calculation model when we take account of the burn-up credit in the spent fuel management. (author)

Overview of safeguards aspects related to MOX fuel

International Nuclear Information System (INIS)

Heinonen, O.J.; Murakami, K.; Shea, T.

2000-01-01

Recent developments in the light of the IAEA verification requirements for MOX fuel at reactors and bulk handling facilities are discussed. Impact of the Additional Protocol and Integrated Safeguards System is briefly addressed. Agency's work undertaken with regard to the nuclear arms control and reduction is presented. (author)

Impact on burnup performance of coated particle fuel design in pebble bed reactor with ROX fuel

International Nuclear Information System (INIS)

Ho, Hai Quan; Obara, Toru

2015-01-01

The pebble bed reactor (PBR), a kind of high-temperature gas-cooled reactor (HTGR), is expected to be among the next generation of nuclear reactors as it has excellent passive safety features, as well as online refueling and high thermal efficiency. Rock-like oxide (ROX) fuel has been studied at the Japan Atomic Energy Agency (JAEA) as a new once-through type fuel concept. Rock-like oxide used as fuel in a PBR can be expected to achieve high burnup and improve chemical stabilities. In the once-through fuel concept, the main challenge is to achieve as high a burnup as possible without failure of the spent fuel. The purpose of this study was to investigate the impact on burnup performance of different coated fuel particle (CFP) designs in a PBR with ROX fuel. In the study, the AGR-1 Coated Particle design and Deep-Burn Coated Particle design were used to make the burnup performance comparison. Criticality and core burnup calculations were performed by MCPBR code using the JENDL-4.0 library. Results at equilibrium showed that the two reactors utilizing AGR-1 Coated Particle and Deep-Burn Coated Particle designs could be critical with almost the same multiplication factor k eff . However, the power peaking factor and maximum power per fuel ball in the AGR-1 coated particle design was lower than that of Deep-Burn coated particle design. The AGR-1 design also showed an advantage in fissions per initial fissile atoms (FIFA); the AGR-1 coated particle design produced a higher FIFA than the Deep-Burn coated particle design. These results suggest that the difference in coated particle fuel design can have an effect on the burnup performance in ROX fuel. (author)

Conversion of highly enriched uranium in thorium-232 based oxide fuel for light water reactors: MOX-T fuel

Energy Technology Data Exchange (ETDEWEB)

Vapirev, E; Jordanov, T; Khristoskov, I [Sofia Univ. (Bulgaria). Fizicheski Fakultet

1996-12-31

The possibility of using highly enriched uranium available from military inventories for production of mixed oxide fuel (MOX) has been proposed. The fuel is based on U-235 dioxide as fissile isotope and Th-232 dioxide as a non-fissile isotope. It is shown that although the fuel conversion coefficient to U-233 is expected to be less than 1, the proposed fuel has several important advantages resulting in cost reduction of the nuclear fuel cycle. The expected properties of MOX fuel (cross-sections, generated chains, delayed neutrons) are estimated. Due to fuel generation the initial enrichment is expected to be 1% less for production of the same energy. In contrast to traditional fuel no long living actinides are generated which reduces the disposal and reprocessing cost. 7 refs.

Burn-up credit in criticality safety of PWR spent fuel

Energy Technology Data Exchange (ETDEWEB)

Mahmoud, Rowayda F., E-mail: Rowayda_mahmoud@yahoo.com [Metallurgy Department, Nuclear Research Center, Atomic Energy Authority (Egypt); Shaat, Mohamed K. [Nuclear Engineering, Reactors Department, Nuclear Research Center, Atomic Energy Authority (Egypt); Nagy, M.E.; Agamy, S.A. [Professor of Nuclear Engineering, Nuclear and Radiation Department, Alexandria University (Egypt); Abdelrahman, Adel A. [Metallurgy Department, Nuclear Research Center, Atomic Energy Authority (Egypt)

2014-12-15

Highlights: • Designing spent fuel wet storage using WIMS-5D and MCNP-5 code. • Studying fresh and burned fuel with/out absorber like “B{sub 4}C and Ag–In–Cd” in racks. • Sub-criticality was confirmed for fresh and burned fuel under specific cases. • Studies for BU credit recommend increasing fuel burn-up to 60.0 GWD/MTU. • Those studies require new core structure materials, fuel composition and cladding. - Abstract: The criticality safety calculations were performed for a proposed design of a wet spent fuel storage pool. This pool will be used for the storage of spent fuel discharged from a typical pressurized water reactor (PWR). The mathematical model based on the international validated codes, WIMS-5 and MCNP-5 were used for calculating the effective multiplication factor, k{sub eff}, for the spent fuel stored in the pool. The data library for the multi-group neutron microscopic cross-sections was used for the cell calculations. The k{sub eff} was calculated for several changes in water density, water level, assembly pitch and burn-up with different initial fuel enrichment and new types and amounts of fixed absorbers. Also, k{sub eff} was calculated for the conservative fresh fuel case. The results of the calculations confirmed that the effective multiplication factor for the spent fuel storage is sub-critical for all normal and abnormal states. The future strategy for the burn-up credit recommends increasing the fuel burn-up to a value >60.0 GWD/MTU, which requires new fuel composition and new fuel cladding material with the assessment of the effects of negative reactivity build up.

Improved locations of reactivity devices in future CANDU reactors fuelled with natural uranium or enriched fuels

International Nuclear Information System (INIS)

Boczar, P.G.; Van Dyk, M.T.

1987-02-01

A new configuration of reactivity devices is proposed for future CANDU reactors which improves the core characteristics with enriched fuels, while still allowing the use of natural uranium fuel. Physics calculations for this new configuration are presented for four fuel types: natural uranium, mixed plutonium - uranium oxide (MOX) having a burnup of 21 MWd/kg, and slightly enriched uranium (SEU) having burnups of either 21 or 31 MWd/kg

Effect of long-term storage of LWR spent fuel on Pu-thermal fuel cycle

International Nuclear Information System (INIS)

Kurosawa, Masayoshi; Naito, Yoshitaka; Suyama, Kenya; Itahara, Kuniyuki; Suzuki, Katsuo; Hamada, Koji

1998-01-01

According to the Long-term Program for Research, Development and Utilization of Nuclear Energy (June, 1994) in Japan, the Rokkasho Reprocessing Plant will be operated shortly after the year 2000, and the planning of the construction of the second commercial plant will be decided around 2010. Also, it is described that spent fuel storage has a positive meaning as an energy resource for the future utilization of Pu. Considering the balance between the increase of spent fuels and the domestic reprocessing capacity in Japan, it can be expected that the long-term storage of UO 2 spent fuels will be required. Then, we studied the effect of long-term storage of spent fuels on Pu-thermal fuel cycle. The burnup calculation were performed on the typical Japanese PWR fuel, and the burnup and criticality calculations were carried out on the Pu-thermal cores with MOX fuel. Based on the results, we evaluate the influence of extending the spent fuel storage term on the criticality safety, shielding design of the reprocessing plant and the core life time of the MOX core, etc. As the result of this work on long-term storage of LWR spent fuels, it becomes clear that there are few demerits regarding the lifetime of a MOX reactor core, and that there are many merits regarding the safety aspects of the fuel cycle facilities. Furthermore, long-term storage is meaningful as energy storage for effective utilization of Pu to be improved by technological innovation in future, and it will allow for sufficient time for the important policymaking of nuclear fuel cycle establishment in Japan. (author)

Nuclear design for high temperature gas cooled reactor (GTHTR300C) using MOX fuel

International Nuclear Information System (INIS)

Mouri, Tomoaki; Kunitomi, Kazuhiko

2008-01-01

A design study of the hydrogen cogeneration high temperature gas cooled reactor (GTHTR300C) that can produce both electricity and hydrogen has been carried out in Japan Atomic Energy Agency. The GTHTR300C is the system with thermal power of 600MW and reactor outlet temperature of 950degC, which is expected to supply the hydrogen to fuel cell vehicles after 2020s. In future, the full deployment of fast reactor cycle without natural uranium will demand the use of Mixed-Oxide (MOX) fuels in the GTHTR300C. Therefore, a nuclear design was performed to confirm the feasibility of the reactor core using MOX fuels. The designed reactor core has high performance and meets safety requirements. In this paper, the outline of the GTHTR300C and the nuclear design of the reactor core using MOX fuels are described. (author)

Nonuniform transformation field analysis of multiphase elasto viscoplastic materials: application to MOX fuels

International Nuclear Information System (INIS)