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Sample records for high-sensitive laser resonance

  1. Highly sensitive high resolution Raman spectroscopy using resonant ionization methods

    International Nuclear Information System (INIS)

    Owyoung, A.; Esherick, P.

    1984-05-01

    In recent years, the introduction of stimulated Raman methods has offered orders of magnitude improvement in spectral resolving power for gas phase Raman studies. Nevertheless, the inherent weakness of the Raman process suggests the need for significantly more sensitive techniques in Raman spectroscopy. In this we describe a new approach to this problem. Our new technique, which we call ionization-detected stimulated Raman spectroscopy (IDSRS), combines high-resolution SRS with highly-sensitive resonant laser ionization to achieve an increase in sensitivity of over three orders of magnitude. The excitation/detection process involves three sequential steps: (1) population of a vibrationally excited state via stimulated Raman pumping; (2) selective ionization of the vibrationally excited molecule with a tunable uv source; and (3) collection of the ionized species at biased electrodes where they are detected as current in an external circuit

  2. Intracavity Laser Photoacoustic Spectrometer with High Sensitivity

    International Nuclear Information System (INIS)

    Mitrayana; Muslim; Wasono, M.A.J.

    2002-01-01

    A photo acoustic spectrometer set-up has been upgraded from an extra cavity into an intracavity configuration using a sealed-off CO 2 laser as the spectrometer's radiation source. The detection level of the upgrade Intracavity Photoacoustic Spectrometer (IPS) reached (200 ± 50) ppt for C 2 H 4 and (20 ± 5) ppt for SF 6 with response time (6.6 ± 0.2) s. (author)

  3. Highly sensitive detection using microring resonator and nanopores

    Science.gov (United States)

    Bougot-Robin, K.; Hoste, J. W.; Le Thomas, N.; Bienstman, P.; Edel, J. B.

    2016-04-01

    One of the most significant challenges facing physical and biological scientists is the accurate detection and identification of single molecules in free-solution environments. The ability to perform such sensitive and selective measurements opens new avenues for a large number of applications in biological, medical and chemical analysis, where small sample volumes and low analyte concentrations are the norm. Access to information at the single or few molecules scale is rendered possible by a fine combination of recent advances in technologies. We propose a novel detection method that combines highly sensitive label-free resonant sensing obtained with high-Q microcavities and position control in nanoscale pores (nanopores). In addition to be label-free and highly sensitive, our technique is immobilization free and does not rely on surface biochemistry to bind probes on a chip. This is a significant advantage, both in term of biology uncertainties and fewer biological preparation steps. Through combination of high-Q photonic structures with translocation through nanopore at the end of a pipette, or through a solid-state membrane, we believe significant advances can be achieved in the field of biosensing. Silicon microrings are highly advantageous in term of sensitivity, multiplexing, and microfabrication and are chosen for this study. In term of nanopores, we both consider nanopore at the end of a nanopipette, with the pore being approach from the pipette with nanoprecise mechanical control. Alternatively, solid state nanopores can be fabricated through a membrane, supporting the ring. Both configuration are discussed in this paper, in term of implementation and sensitivity.

  4. New laser system for highly sensitive clinical pulse oximetry

    Science.gov (United States)

    Hamza, Mostafa; Hamza, Mohammad

    1996-04-01

    This paper describes the theory and design of a new pulse oximeter in which laser diodes and other compact laser sources are used for the measurement of oxygen saturation in patients who are at risk of developing hypoxemia. The technique depends upon illuminating special sites of the skin of the patient with radiation from modulated laser sources at selected wavelengths. The specific laser wavelengths are chosen based on the absorption characteristics of oxyhemoglobin, reduced hemoglobin and other interfering sources for obtaining more accurate measurements. The laser radiation transmitted through the tissue is detected and signal processing based on differential absorption laser spectroscopy is done in such a way to overcome the primary performance limitations of the conventionally used pulse oximetry. The new laser pulse oximeter can detect weak signals and is not affected by other light sources such as surgical lamps, phototherapy units, etc. The detailed description and operating characteristics of this system are presented.

  5. Real-time, single-step bioassay using nanoplasmonic resonator with ultra-high sensitivity

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, Xiang; Ellman, Jonathan A; Chen, Fanqing Frank; Su, Kai-Hang; Wei, Qi-Huo; Sun, Cheng

    2014-04-01

    A nanoplasmonic resonator (NPR) comprising a metallic nanodisk with alternating shielding layer(s), having a tagged biomolecule conjugated or tethered to the surface of the nanoplasmonic resonator for highly sensitive measurement of enzymatic activity. NPRs enhance Raman signals in a highly reproducible manner, enabling fast detection of protease and enzyme activity, such as Prostate Specific Antigen (paPSA), in real-time, at picomolar sensitivity levels. Experiments on extracellular fluid (ECF) from paPSA-positive cells demonstrate specific detection in a complex bio-fluid background in real-time single-step detection in very small sample volumes.

  6. High resolution laser spectroscopy of the D lines of on-line produced 21Na, 22Na, 24Na, 25Na using a new high sensitivity method of detection of optical resonances

    International Nuclear Information System (INIS)

    Huber, G.; Thibault, G.; Klapisch, R.; Duong, H.T.; Vialle, J.L.; Pinard, I.; Juncar, P.; Jacquinot, P.

    1975-01-01

    A polyisotopic sodium beam of 21 - 25 Na, produced by spallation of Al, was illuminated by a tunable dye laser. The atomic beam, analyzed by a sixpole magnet is then ionized and detected after a mass spectrometer. The results are the isotope shifts, nuclear magnetic moment and quadrupole moment of 25 Na [fr

  7. Laser magnetic resonance spectroscopy

    International Nuclear Information System (INIS)

    Ferrari, C.A.

    1985-01-01

    The technique of laser resonance magnetic resonance allows one to study the high-resolution spectroscopy of transient paramagnetic species, viz, atoms, radicals, and molecular ions. This article is a brief exposition of the method, describing the principles, instrumentation and applicability of the IR and FIR-LMR and shows results of HF + . (Author) [pt

  8. Highly Sensitive Measurement of Liquid Density in Air Using Suspended Microcapillary Resonators

    Directory of Open Access Journals (Sweden)

    Oscar Malvar

    2015-03-01

    Full Text Available We report the use of commercially available glass microcapillaries as micromechanical resonators for real-time monitoring of the mass density of a liquid that flows through the capillary. The vibration of a suspended region of the microcapillary is optically detected by measuring the forward scattering of a laser beam. The resonance frequency of the liquid filled microcapillary is measured for liquid binary mixtures of ethanol in water, glycerol in water and Triton in ethanol. The method achieves a detection limit in an air environment of 50 µg/mL that is only five times higher than that obtained with state-of-the-art suspended microchannel resonators encapsulated in vacuum. The method opens the door to novel advances for miniaturized total analysis systems based on microcapillaries with the add-on of mechanical transduction for sensing the rheological properties of the analyzed fluids without the need for vacuum encapsulation of the resonators.

  9. Resonant laser ablation: mechanisms and applications

    International Nuclear Information System (INIS)

    Anderson, J.E.; Bodla, R.; Eiden, G.C.; Nogar, N.S.; Smith, C.H.

    1996-01-01

    Resonant laser ablation (RLA) typically relies on irradiation of a sample in a mass spectrometer with modest intensity laser pulses tuned to a one or two photon resonant transition in the analyte of interest. This paper shows that RLA is well suited for highly sensitive analyses of complex samples. The examples actually studied are trace components in rhenium and technetium in nickel. The authors also studied the 2+1 multiphoton ionization spectrum of iron-56 detected by RLA of Re containing 70 ppm iron. Two-photon transition rates for Fe transitions were calculated perturbatively and found to agree semi-quantitatively with experimentally observed intensities. 17 refs., 3 figs

  10. High sensitivity detection of selenium by laser excited atomic fluorescence spectrometry using electrothermal atomization

    International Nuclear Information System (INIS)

    Heitmann, U.; Hese, A.; Schoknecht, G.; Gries, W.

    1995-01-01

    The high sensitivity detection of the trace element selenium is reported. The analytical method applied is Laser Excited Atomic Fluorescence Spectrometry using Electrothermal Atomization within a graphite furnace atomizer. For the production of tunable laser radiation in the VUV spectral region a laser system was developed which consists of two dye lasers pumped by a Nd:YAG laser. The laser radiations are subsequently frequency doubled and sum frequency mixed by nonlinear optical KDP or BBO crystals, respectively. The system works with a repetition rate of 20 Hz and provides output energies of up to 100 μJ in the VUV at a pulse duration of 5 ns. The analytical investigations were focused on the detection of selenium in aqueous solutions and samples of human whole blood. From measurements on aqueous standards detection limits of 1.5 ng/l for selenium were obtained, with corresponding absolute detected masses of only 15 fg. The linear dynamic range spanned six orders of magnitude and good precision was achieved. In case of human whole blood samples the recovery was found to be within the range of 96% to 104%. The determination of the selenium content yielded medians of [119.5 ± 17.3] μg/l for 200 frozen blood samples taken in 1988 and [109.1 ± 15.6] μg/l for 103 fresh blood samples. (author)

  11. Injection-controlled laser resonator

    Science.gov (United States)

    Chang, J.J.

    1995-07-18

    A new injection-controlled laser resonator incorporates self-filtering and self-imaging characteristics with an efficient injection scheme. A low-divergence laser signal is injected into the resonator, which enables the injection signal to be converted to the desired resonator modes before the main laser pulse starts. This injection technique and resonator design enable the laser cavity to improve the quality of the injection signal through self-filtering before the main laser pulse starts. The self-imaging property of the present resonator reduces the cavity induced diffraction effects and, in turn, improves the laser beam quality. 5 figs.

  12. Highly sensitive nano-porous lattice biosensor based on localized surface plasmon resonance and interference.

    Science.gov (United States)

    Yeom, Se-Hyuk; Kim, Ok-Geun; Kang, Byoung-Ho; Kim, Kyu-Jin; Yuan, Heng; Kwon, Dae-Hyuk; Kim, Hak-Rin; Kang, Shin-Won

    2011-11-07

    We propose a design for a highly sensitive biosensor based on nanostructured anodized aluminum oxide (AAO) substrates. A gold-deposited AAO substrate exhibits both optical interference and localized surface plasmon resonance (LSPR). In our sensor, application of these disparate optical properties overcomes problems of limited sensitivity, selectivity, and dynamic range seen in similar biosensors. We fabricated uniform periodic nanopore lattice AAO templates by two-step anodizing and assessed their suitability for application in biosensors by characterizing the change in optical response on addition of biomolecules to the AAO template. To determine the suitability of such structures for biosensing applications, we immobilized a layer of C-reactive protein (CRP) antibody on a gold coating atop an AAO template. We then applied a CRP antigen (Ag) atop the immobilized antibody (Ab) layer. The shift in reflectance is interpreted as being caused by the change in refractive index with membrane thickness. Our results confirm that our proposed AAO-based biosensor is highly selective toward detection of CRP antigen, and can measure a change in CRP antigen concentration of 1 fg/ml. This method can provide a simple, fast, and sensitive analysis for protein detection in real-time.

  13. Laser cooling at resonance

    Science.gov (United States)

    Yudkin, Yaakov; Khaykovich, Lev

    2018-05-01

    We show experimentally that three-dimensional laser cooling of lithium atoms on the D2 line is possible when the laser light is tuned exactly to resonance with the dominant atomic transition. Qualitatively, it can be understood by applying simple Doppler cooling arguments to the specific hyperfine structure of the excited state of lithium atoms, which is both dense and inverted. However, to build a quantitative theory, we must resolve to a full model which takes into account both the entire atomic structure of all 24 Zeeman sublevels and the laser light polarization. Moreover, by means of Monte Carlo simulations, we show that coherent processes play an important role in showing consistency between the theory and the experimental results.

  14. A flexible and highly sensitive nonenzymatic glucose sensor based on DVD-laser scribed graphene substrate.

    Science.gov (United States)

    Lin, Songyue; Feng, Wendou; Miao, Xiaofei; Zhang, Xiangxin; Chen, Sujing; Chen, Yuanqiang; Wang, Wei; Zhang, Yining

    2018-07-01

    Flexible and implantable glucose biosensors are emerging technologies for continuous monitoring of blood-glucose of diabetes. Developing a flexible conductive substrates with high active surface area is critical for advancing the technology. Here, we successfully fabricate a flexible and highly sensitive nonenzymatic glucose by using DVD-laser scribed graphene (LSG) as a flexible conductively substrate. Copper nanoparticles (Cu-NPs) are electrodeposited as the catalyst. The LSG/Cu-NPs sensor demonstrates excellent catalytic activity toward glucose oxidation and exhibits a linear glucose detection range from 1 μM to 4.54 mM with high sensitivity (1.518 mA mM -1 cm -2 ) and low limit of detection (0.35 μM). Moreover, the LSG/Cu-NPs sensor shows excellent reproducibility and long-term stability. It is also highly selective toward glucose oxidation under the presence of various interfering species. Excellent flexing stability is also demonstrated by the LSG/Cu-NPs sensor, which is capable of maintaining 83.9% of its initial current after being bent against a 4-mm diameter rod for 180 times. The LSG/Cu-NPs sensor shows great potential for practical application as a nonenzymatic glucose biosensor. Meanwhile, the LSG conductive substrate provides a platform for the developing next-generation flexible and potentially implantable bioelectronics and biosensors. Copyright © 2018 Elsevier B.V. All rights reserved.

  15. A car-borne highly sensitive near-IR diode-laser methane detector

    International Nuclear Information System (INIS)

    Berezin, A G; Ershov, Oleg V; Shapovalov, Yu P

    2003-01-01

    A highly sensitive automated car-borne detector for measuring methane concentration in real time is designed, developed and tested under laboratory and field conditions. Measurements were made with the help of an uncooled tunable near-IR 1.65-μm laser diode. The detector consists of a multipass optical cell with a 45-m long optical path and a base length of 0.5 m. The car-borne detector is intended for monitoring the methane concentration in air from the moving car to reveal the leakage of domestic gas. The sensitivity limit (standard deviation) under field conditions is 1 ppm (20 ppb under laboratory conditions) for a measuring time of 0.4 s. The measuring technique based on the detection of a single methane line ensured a high selectivity of methane detector relative to other gases. The methane detector can be easily modified for measuring other simple-molecule gases (e.g., CO, CO 2 , HF, NO 2 , H 2 O) by replacing the diode laser and varying the parameters of the control program. (special issue devoted to the memory of academician a m prokhorov)

  16. Highly Sensitive Tunable Diode Laser Spectrometers for In Situ Planetary Exploration

    Science.gov (United States)

    Vasudev, Ram; Mansour, Kamjou; Webster, Christopher R.

    2013-01-01

    This paper describes highly sensitive tunable diode laser spectrometers suitable for in situ planetary exploration. The technology developed at JPL is based on wavelength modulated cavity enhanced absorption spectroscopy. It is capable of sensitively detecting chemical signatures of life through the abundance of biogenic molecules and their isotopic composition, and chemicals such as water necessary for habitats of life. The technology would be suitable for searching for biomarkers, extinct life, potential habitats of extant life, and signatures of ancient climates on Mars; and for detecting biomarkers, prebiotic chemicals and habitats of life in the outer Solar System. It would be useful for prospecting for water on the Moon and asteroids, and characterizing its isotopic composition. Deployment on the Moon could provide ground truth to the recent remote measurements and help to uncover precious records of the early bombardment history of the inner Solar System buried at the shadowed poles, and elucidate the mechanism for the generation of near-surface water in the illuminated regions. The technology would also be useful for detecting other volatile molecules in planetary atmospheres and subsurface reservoirs, isotopic characterization of planetary materials, and searching for signatures of extinct life preserved in solid matrices.

  17. Resonance Ionization Laser Ion Sources

    CERN Document Server

    Marsh, B

    2013-01-01

    The application of the technique of laser resonance ionization to the production of singly charged ions at radioactive ion beam facilities is discussed. The ability to combine high efficiency and element selectivity makes a resonance ionization laser ion source (RILIS) an important component of many radioactive ion beam facilities. At CERN, for example, the RILIS is the most commonly used ion source of the ISOLDE facility, with a yearly operating time of up to 3000 hours. For some isotopes the RILIS can also be used as a fast and sensitive laser spectroscopy tool, provided that the spectral resolution is sufficiently high to reveal the influence of nuclear structure on the atomic spectra. This enables the study of nuclear properties of isotopes with production rates even lower than one ion per second and, in some cases, enables isomer selective ionization. The solutions available for the implementation of resonance laser ionization at radioactive ion beam facilities are summarized. Aspects such as the laser r...

  18. Surface plasmon resonance biosensors for highly sensitive detection in real samples

    Science.gov (United States)

    Sepúlveda, B.; Carrascosa, L. G.; Regatos, D.; Otte, M. A.; Fariña, D.; Lechuga, L. M.

    2009-08-01

    In this work we summarize the main results obtained with the portable surface plasmon resonance (SPR) device developed in our group (commercialised by SENSIA, SL, Spain), highlighting its applicability for the real-time detection of extremely low concentrations of toxic pesticides in environmental water samples. In addition, we show applications in clinical diagnosis as, on the one hand, the real-time and label-free detection of DNA hybridization and single point mutations at the gene BRCA-1, related to the predisposition in women to develop an inherited breast cancer and, on the other hand, the analysis of protein biomarkers in biological samples (urine, serum) for early detection of diseases. Despite the large number of applications already proven, the SPR technology has two main drawbacks: (i) not enough sensitivity for some specific applications (where pM-fM or single-molecule detection are needed) (ii) low multiplexing capabilities. In order solve such drawbacks, we work in several alternative configurations as the Magneto-optical Surface Plasmon Resonance sensor (MOSPR) based on a combination of magnetooptical and ferromagnetic materials, to improve the SPR sensitivity, or the Localized Surface Plasmon Resonance (LSPR) based on nanostructures (nanoparticles, nanoholes,...), for higher multiplexing capabilities.

  19. High-sensitivity dc field magnetometer using nonlinear resonance magnetoelectric effect

    International Nuclear Information System (INIS)

    Burdin, D.A.; Chashin, D.V.; Ekonomov, N.A.; Fetisov, Y.K.; Stashkevich, A.A.

    2016-01-01

    The design and operation principle of dc field magnetometer using nonlinear resonance magnetoelectric effect in a ferromagnetic–piezoelectric structure are described. It is shown that under action of ac pumping magnetic field the structure generates the output voltage containing higher harmonics whose amplitudes depend on the dc magnetic field. Best performance of the device is obtained if the signal of the third harmonics is used for the dc field measurement. The sensitivity can be considerably (by approximately three orders of magnitude) increased if advantage is taken of the acoustic resonance of the structure at this frequency. There exists the optimal pumping field ensuring the highest sensitivity. Further increasing of this field expands the range of measurable dc fields at the expense of deteriorated sensitivity. The magnetometer fabricated on the basis of a planar langatate-Metglas structure had sensitivity up to ~1 V/Oe and allowed detection of the fields as low as ~10"−"5 Oe. - Highlights: • Operational principle and design of new type dc field magnetometer is described. • Magnetometer uses nonlinear magnetoelectric effect in a langatate-Metglas structure. • Magnetometer has sensitivity of ~1 V/Oe and detects fields as low as 10"−"5 Oe. • The proposed magnetometer can compete with well known fluxgate sensors.

  20. High-sensitivity dc field magnetometer using nonlinear resonance magnetoelectric effect

    Energy Technology Data Exchange (ETDEWEB)

    Burdin, D.A.; Chashin, D.V.; Ekonomov, N.A. [Moscow State University of Information Technologies, Radio Engineering and Electronics, Moscow (Russian Federation); Fetisov, Y.K., E-mail: fetisov@mirea.ru [Moscow State University of Information Technologies, Radio Engineering and Electronics, Moscow (Russian Federation); Stashkevich, A.A. [LSPM (CNRS-UPR 3407), Université Paris 13, Sorbonne Paris Cité, 93430 Villetaneuse (France)

    2016-05-01

    The design and operation principle of dc field magnetometer using nonlinear resonance magnetoelectric effect in a ferromagnetic–piezoelectric structure are described. It is shown that under action of ac pumping magnetic field the structure generates the output voltage containing higher harmonics whose amplitudes depend on the dc magnetic field. Best performance of the device is obtained if the signal of the third harmonics is used for the dc field measurement. The sensitivity can be considerably (by approximately three orders of magnitude) increased if advantage is taken of the acoustic resonance of the structure at this frequency. There exists the optimal pumping field ensuring the highest sensitivity. Further increasing of this field expands the range of measurable dc fields at the expense of deteriorated sensitivity. The magnetometer fabricated on the basis of a planar langatate-Metglas structure had sensitivity up to ~1 V/Oe and allowed detection of the fields as low as ~10{sup −5} Oe. - Highlights: • Operational principle and design of new type dc field magnetometer is described. • Magnetometer uses nonlinear magnetoelectric effect in a langatate-Metglas structure. • Magnetometer has sensitivity of ~1 V/Oe and detects fields as low as 10{sup −5} Oe. • The proposed magnetometer can compete with well known fluxgate sensors.

  1. A cyclotron resonance laser accelerator

    International Nuclear Information System (INIS)

    Sprangle, P.; Tang, C.M.; Vlahos, L.

    1983-01-01

    A laser acceleration mechanism which utilizes a strong static, almost uniform, magnetic field together with an intense laser pulse is analyzed. The interaction and acceleration mechanism relies on a self resonance effect. Since the laser field is assumed to be diffraction limited, the magnetic field must be spatially varied to maintain resonance. The effective accelerating gradient is shown to scale like 1/√E /SUB b/ , where E /SUB b/ is the electron energy. For a numerical illustration the authors consider a 1 x 10 13 W/cm 2 , CO 2 laser and show that electrons can be accelerated to more than 500 MeV in a distance of 15 m (approximately two Rayleigh lengths)

  2. Pulsed laser deposition of Ag nanoparticles on titanium hydroxide/oxide nanobelt arrays for highly sensitive surface-enhanced Raman spectroscopy

    International Nuclear Information System (INIS)

    Jing, Yuting; Wang, Huanwen; Zhao, Jie; Yi, Huan; Wang, Xuefeng

    2015-01-01

    Highlights: • Silver nanoparticles (NPs) were deposited on Ti(OH) 4 nanobelt by pulsed laser deposition (PLD). • The highest enhancement factor of 10 6 and a maximum relative standard deviation (RSD) of 0.18. • Ag 2 O play important role for the high sensitivity Raman phenomenon. • Charge transfer from Ag NPs is also responsible for the enhancement ability. - Abstract: Surface-enhanced Raman scattering (SERS) substrate of Ti(OH) 4 nanobelt arrays (NBAs) was synthesized by a hydrothermal reaction, on which silver nanoparticles (NPs) were deposited by pulsed laser deposition (PLD). Field-emission scanning electron microscopy (FESEM) and transmission electron microscopy (TEM) revealed the effective high specific surface area with silver NPs decorated on three-dimensional NBAs. Using rhodamine 6G (R6G) as an analyte molecule, the highest enhancement factor of 10 6 and a maximum relative standard deviation (RSD) of 0.18 were obtained. It has been found that the specific morphology of these composite nanobelt arrays and the formation of Ag 2 O play important role for the high sensitivity Raman phenomenon. In addition, the surface plasmon resonance wavelength of Ag decorated Ti(OH) 4 NBAs and the charge transfer from Ag NPs are also responsible for the enhancement ability. For comparison SERS was investigated with silver particles decorated on TiO 2 NBAs, which is much less active

  3. Laser-engraved carbon nanotube paper for instilling high sensitivity, high stretchability, and high linearity in strain sensors

    KAUST Repository

    Xin, Yangyang

    2017-06-29

    There is an increasing demand for strain sensors with high sensitivity and high stretchability for new applications such as robotics or wearable electronics. However, for the available technologies, the sensitivity of the sensors varies widely. These sensors are also highly nonlinear, making reliable measurement challenging. Here we introduce a new family of sensors composed of a laser-engraved carbon nanotube paper embedded in an elastomer. A roll-to-roll pressing of these sensors activates a pre-defined fragmentation process, which results in a well-controlled, fragmented microstructure. Such sensors are reproducible and durable and can attain ultrahigh sensitivity and high stretchability (with a gauge factor of over 4.2 × 10(4) at 150% strain). Moreover, they can attain high linearity from 0% to 15% and from 22% to 150% strain. They are good candidates for stretchable electronic applications that require high sensitivity and linearity at large strains.

  4. Palladium Nanoparticles-Based Fluorescence Resonance Energy Transfer Aptasensor for Highly Sensitive Detection of Aflatoxin M₁ in Milk.

    Science.gov (United States)

    Li, Hui; Yang, Daibin; Li, Peiwu; Zhang, Qi; Zhang, Wen; Ding, Xiaoxia; Mao, Jin; Wu, Jing

    2017-10-13

    A highly sensitive aptasensor for aflatoxin M₁ (AFM₁) detection was constructed based on fluorescence resonance energy transfer (FRET) between 5-carboxyfluorescein (FAM) and palladium nanoparticles (PdNPs). PdNPs (33 nm) were synthesized through a seed-mediated growth method and exhibited broad and strong absorption in the whole ultraviolet-visible (UV-Vis) range. The strong coordination interaction between nitrogen functional groups of the AFM₁ aptamer and PdNPs brought FAM and PdNPs in close proximity, which resulted in the fluorescence quenching of FAM to a maximum extent of 95%. The non-specific fluorescence quenching caused by PdNPs towards fluorescein was negligible. After the introduction of AFM₁ into the FAM-AFM₁ aptamer-PdNPs FRET system, the AFM₁ aptamer preferentially combined with AFM₁ accompanied by conformational change, which greatly weakened the coordination interaction between the AFM₁ aptamer and PdNPs. Thus, fluorescence recovery of FAM was observed and a linear relationship between the fluorescence recovery and the concentration of AFM₁ was obtained in the range of 5-150 pg/mL in aqueous buffer with the detection limit of 1.5 pg/mL. AFM₁ detection was also realized in milk samples with a linear detection range from 6 pg/mL to 150 pg/mL. The highly sensitive FRET aptasensor with simple configuration shows promising prospect in detecting a variety of food contaminants.

  5. Fabrication and characterization of gold nanocrown arrays on a gold film for a high-sensitivity surface plasmon resonance biosensor

    Energy Technology Data Exchange (ETDEWEB)

    Choi, Munsik; Kim, Nak-hyeon; Eom, Seyoung [Department of Biomedical Engineering, Kyung Hee University, Yongin 446-701 (Korea, Republic of); Kim, Tae Woo [School of East–West Medical Science, Kyung Hee University, Yongin 446-701 (Korea, Republic of); Byun, Kyung Min, E-mail: kmbyun@khu.ac.kr [Department of Biomedical Engineering, Kyung Hee University, Yongin 446-701 (Korea, Republic of); Park, Hyeong-Ho, E-mail: hyeongho.park@kanc.re.kr [Nano Process Division, Korea Advanced Nano Fab Center, Suwon 443-270 (Korea, Republic of)

    2015-07-31

    We report on a versatile method to fabricate gold nanocrown arrays on a thin gold film based on ultraviolet nanoimprint lithography and tilted evaporation technique. We realize highly ordered 2-dimensional nanocrown arrays and characterize their sizes and morphologies using scanning electron microscopy. To demonstrate an enhanced surface plasmon resonance (SPR) detection by the fabricated gold nanocrown samples, biosensing experiments are performed by measuring SPR angle shift for biotin–streptavidin interaction and bulk refractive index change of dielectric medium. We hope that the suggested plasmonic platform with a high sensitivity could be extended to a variety of biomolecular binding reactions. - Highlights: • Gold nanocrown arrays are produced by nanoimprint lithography and tilted evaporation. • Use of gold nanocrown arrays can improve the sensor sensitivity significantly. • Improved sensitivity is due to enhanced field–matter interaction at gold nanocrowns.

  6. Highly sensitive refractive index fiber inline Mach-Zehnder interferometer fabricated by femtosecond laser micromachining and chemical etching

    Science.gov (United States)

    Sun, Xiao-Yan; Chu, Dong-Kai; Dong, Xin-Ran; Zhou, Chu; Li, Hai-Tao; Luo-Zhi; Hu, You-Wang; Zhou, Jian-Ying; Cong-Wang; Duan, Ji-An

    2016-03-01

    A High sensitive refractive index (RI) sensor based on Mach-Zehnder interferometer (MZI) in a conventional single-mode optical fiber is proposed, which is fabricated by femtosecond laser transversal-scanning inscription method and chemical etching. A rectangular cavity structure is formed in part of fiber core and cladding interface. The MZI sensor shows excellent refractive index sensitivity and linearity, which exhibits an extremely high RI sensitivity of -17197 nm/RIU (refractive index unit) with the linearity of 0.9996 within the refractive index range of 1.3371-1.3407. The experimental results are consistent with theoretical analysis.

  7. High-speed high-sensitivity infrared spectroscopy using mid-infrared swept lasers (Conference Presentation)

    Science.gov (United States)

    Childs, David T. D.; Groom, Kristian M.; Hogg, Richard A.; Revin, Dmitry G.; Cockburn, John W.; Rehman, Ihtesham U.; Matcher, Stephen J.

    2016-03-01

    Infrared spectroscopy is a highly attractive read-out technology for compositional analysis of biomedical specimens because of its unique combination of high molecular sensitivity without the need for exogenous labels. Traditional techniques such as FTIR and Raman have suffered from comparatively low speed and sensitivity however recent innovations are challenging this situation. Direct mid-IR spectroscopy is being speeded up by innovations such as MEMS-based FTIR instruments with very high mirror speeds and supercontinuum sources producing very high sample irradiation levels. Here we explore another possible method - external cavity quantum cascade lasers (EC-QCL's) with high cavity tuning speeds (mid-IR swept lasers). Swept lasers have been heavily developed in the near-infrared where they are used for non-destructive low-coherence imaging (OCT). We adapt these concepts in two ways. Firstly by combining mid-IR quantum cascade gain chips with external cavity designs adapted from OCT we achieve spectral acquisition rates approaching 1 kHz and demonstrate potential to reach 100 kHz. Secondly we show that mid-IR swept lasers share a fundamental sensitivity advantage with near-IR OCT swept lasers. This makes them potentially able to achieve the same spectral SNR as an FTIR instrument in a time x N shorter (N being the number of spectral points) under otherwise matched conditions. This effect is demonstrated using measurements of a PDMS sample. The combination of potentially very high spectral acquisition rates, fundamental SNR advantage and the use of low-cost detector systems could make mid-IR swept lasers a powerful technology for high-throughput biomedical spectroscopy.

  8. Silica Gel Coated Spherical Micro resonator for Ultra-High Sensitivity Detection of Ammonia Gas Concentration in Air.

    Science.gov (United States)

    Mallik, Arun Kumar; Farrell, Gerald; Liu, Dejun; Kavungal, Vishnu; Wu, Qiang; Semenova, Yuliya

    2018-01-26

    A silica gel coated microsphere resonator is proposed and experimentally demonstrated for measurements of ammonia (NH 3 ) concentration in air with ultra-high sensitivity. The optical properties of the porous silica gel layer change when it is exposed to low (parts per million (ppm)) and even ultra-low (parts per billion (ppb)) concentrations of ammonia vapor, leading to a spectral shift of the WGM resonances in the transmission spectrum of the fiber taper. The experimentally demonstrated sensitivity of the proposed sensor to ammonia is estimated as 34.46 pm/ppm in the low ammonia concentrations range from 4 ppm to 30 ppm using an optical spectrum analyser (OSA), and as 800 pm/ppm in the ultra-low range of ammonia concentrations from 2.5 ppb to 12 ppb using the frequency detuning method, resulting in the lowest detection limit (by two orders of magnitude) reported to date equal to 0.16 ppb of ammonia in air. In addition, the sensor exhibits excellent selectivity to ammonia and very fast response and recovery times measured at 1.5 and 3.6 seconds, respectively. Other attractive features of the proposed sensor are its compact nature, simplicity of fabrication.

  9. Highly sensitive SnO2 sensor via reactive laser-induced transfer

    Science.gov (United States)

    Palla Papavlu, Alexandra; Mattle, Thomas; Temmel, Sandra; Lehmann, Ulrike; Hintennach, Andreas; Grisel, Alain; Wokaun, Alexander; Lippert, Thomas

    2016-04-01

    Gas sensors based on tin oxide (SnO2) and palladium doped SnO2 (Pd:SnO2) active materials are fabricated by a laser printing method, i.e. reactive laser-induced forward transfer (rLIFT). Thin films from tin based metal-complex precursors are prepared by spin coating and then laser transferred with high resolution onto sensor structures. The devices fabricated by rLIFT exhibit low ppm sensitivity towards ethanol and methane as well as good stability with respect to air, moisture, and time. Promising results are obtained by applying rLIFT to transfer metal-complex precursors onto uncoated commercial gas sensors. We could show that rLIFT onto commercial sensors is possible if the sensor structures are reinforced prior to printing. The rLIFT fabricated sensors show up to 4 times higher sensitivities then the commercial sensors (with inkjet printed SnO2). In addition, the selectivity towards CH4 of the Pd:SnO2 sensors is significantly enhanced compared to the pure SnO2 sensors. Our results indicate that the reactive laser transfer technique applied here represents an important technical step for the realization of improved gas detection systems with wide-ranging applications in environmental and health monitoring control.

  10. High-sensitivity high-selectivity detection of CWAs and TICs using tunable laser photoacoustic spectroscopy

    Science.gov (United States)

    Pushkarsky, Michael; Webber, Michael; Patel, C. Kumar N.

    2005-03-01

    We provide a general technique for evaluating the performance of an optical sensor for the detection of chemical warfare agents (CWAs) in realistic environments and present data from a simulation model based on a field deployed discretely tunable 13CO2 laser photoacoustic spectrometer (L-PAS). Results of our calculations show the sensor performance in terms of usable sensor sensitivity as a function of probability of false positives (PFP). The false positives arise from the presence of many other gases in the ambient air that could be interferents. Using the L-PAS as it exists today, we can achieve a detection threshold of about 4 ppb for the CWAs while maintaining a PFP of less than 1:106. Our simulation permits us to vary a number of parameters in the model to provide guidance for performance improvement. We find that by using a larger density of laser lines (such as those obtained through the use of tunable semiconductor lasers), improving the detector noise and maintaining the accuracy of laser frequency determination, optical detection schemes can make possible CWA sensors having sub-ppb detection capability with TIC detection.

  11. Highly Sensitive TGA Diagnosis of Thermal Behaviour of Laser-Deposited Materials

    Czech Academy of Sciences Publication Activity Database

    Galíková, Anna; Pola, Josef

    2008-01-01

    Roč. 473, 1-2 (2008), s. 54-60 ISSN 0040-6031 R&D Projects: GA AV ČR IAA400720619 Institutional research plan: CEZ:AV0Z40720504 Keywords : thermogravimetry * laser-deposited materials * mass spectroscopy Subject RIV: CF - Physical ; Theoretical Chemistry Impact factor: 1.659, year: 2008

  12. High sensitivity spectroscopy with tunable diode lasers - detection of O2 quadrupole transitions and 14C

    International Nuclear Information System (INIS)

    Reid, J.

    1981-01-01

    In recent years, tunable lead-salt diode lasers (TDLs) have found widespread application in all fields of infrared spectroscopy. However, most applications of TDLs utilise only the tunability and high resolution of these devices, and few experiments have employed the ability of the TDL to detect very small absorption coefficients. We have developed a laser absorption spectrometer (LAS) which can detect absorption coefficients as small as 10 -6 to 10 -7 m -1 , while retaining the full tunability and resolution of the TDL. This instrument has been used as a point monitoring system for many trace gases of atmospheric significance. In this paper, we describe two additional applications of the LAS: (I) the detection of very weak transitions such as quadrupole lines in oxygen, and (II) the detection of rare isotopes, with 14 C in CO 2 as an example. Details are given in the following sections. (orig.)

  13. A new high sensitivity far-infrared laser interferometer for the HL-2A tokamak

    Science.gov (United States)

    Li, Y. G.; Zhou, Y.; Li, Y.; Deng, Z. C.; Wang, H. X.; Yi, J.

    2017-08-01

    A new four-chord Michelson-type formic acid (HCOOH, λ = 432.5 μm) laser interferometer has been successfully commissioned on the HL-2A tokamak to measure the electron density and density fluctuations. Due to the employment of the two-laser heterodyne technique, the time resolution of the interferometer reached 1.0 microseconds (μs). Four chords of line electron densities with a line-averaged density resolution 2 × 1016/m3 were obtained in a recent HL-2A experimental campaign, and detailed electron density fluctuations, caused by events such as edge localized mode, sawtooth precursor-oscillations, and energetic particle driven instabilities, were distinctly measured. In particular, the high-frequency electron density fluctuations (up to 500 kHz) caused by the reversed shear Alfvénic eigenmode were observed by the internal two interferometry channels, and their fluctuation location could be approximately identified from the spectra characteristics of multi-chord line electron densities.

  14. Laser photoacoustic spectroscopy helps fight terrorism: High sensitivity detection of chemical Warfare Agent and explosives

    Science.gov (United States)

    Patel, C. K. N.

    2008-01-01

    Tunable laser photoacoustic spectroscopy is maturing rapidly in its applications to real world problems. One of the burning problems of the current turbulent times is the threat of terrorist acts against civilian population. This threat appears in two distinct forms. The first is the potential release of chemical warfare agents (CWA), such as the nerve agents, in a crowded environment. An example of this is the release of Sarin by Aum Shinrikyo sect in a crowded Tokyo subway in 1995. An example of the second terrorist threat is the ever-present possible suicide bomber in crowded environment such as airports, markets and large buildings. Minimizing the impact of both of these threats requires early detection of the presence of the CWAs and explosives. Photoacoustic spectroscopy is an exquisitely sensitive technique for the detection of trace gaseous species, a property that Pranalytica has extensively exploited in its CO2 laser based commercial instrumentation for the sub-ppb level detection of a number of industrially important gases including ammonia, ethylene, acrolein, sulfur hexafluoride, phosphine, arsine, boron trichloride and boron trifluoride. In this presentation, I will focus, however, on our recent use of broadly tunable single frequency high power room temperature quantum cascade lasers (QCL) for the detection of the CWAs and explosives. Using external grating cavity geometry, we have developed room temperature QCLs that produce continuously tunable single frequency CW power output in excess of 300 mW at wavelengths covering 5 μm to 12 μm. I will present data that show a CWA detection capability at ppb levels with false alarm rates below 1:108. I will also show the capability of detecting a variety of explosives at a ppb level, again with very low false alarm rates. Among the explosives, we have demonstrated the capability of detecting homemade explosives such as triacetone triperoxide and its liquid precursor, acetone which is a common household

  15. High-sensitive nitrogen dioxide and ethanol gas sensor using a reduced graphene oxide-loaded double split ring resonator

    Science.gov (United States)

    Singh, Sandeep Kumar; Azad, Prakrati; Akhtar, M. J.; Kar, Kamal K.

    2017-08-01

    A reduced graphene oxide (rGO) incorporated double split ring resonator (DSRR) portable microwave gas sensor is proposed in this work. The sensor is fabricated using two major steps: the DSRR is fabricated on the FR-4 substrate, which is excited by a high impedance microstrip line. The rGO is synthesized via a chemical route and coated inside the smaller ring of the DSRR. The SEM micrographs reveal crumpled sheets of rGO that provide a large surface area, and the XRD patterns of the as-synthesized rGO reveal the two-dimensional structure of the rGO nanosheets. The sensor performance is measured at room temperature using 100-400 ppm of ethanol and NO2 target gases. At 400 ppm, the sensor reveals a shift of 420 and 390 MHz in the S 21 frequency for NO2 and ethanol gases, respectively. The frequency shifts of 130 and 120 MHz in the S 21 resonance frequency are obtained for NO2 and ethanol gases, respectively, at a very low concentration of 100 ppm. The high sensitivity of the proposed rGO gas sensor is achieved due to the combined effect of the large surface area of the rGO responsible for accommodating more gas molecules, and its increased conductivity due to the transfer of the electron from the rGO. Moreover, an exceedingly short response time is observed for NO2 in comparison to ethanol, which allows the proposed sensor to be used for the selective detection of NO2 in a harsh environment. The overall approach used in this study is quite simple, and has great potential to enhance the gas detection behaviour of rGO.

  16. Electron spin resonance as a high sensitivity technique for environmental magnetism: determination of contamination in carbonate sediments

    Science.gov (United States)

    Crook, Nigel P.; Hoon, Stephen R.; Taylor, Kevin G.; Perry, Chris T.

    2002-05-01

    This study investigates the application of high sensitivity electron spin resonance (ESR) to environmental magnetism in conjunction with the more conventional techniques of magnetic susceptibility, vibrating sample magnetometry (VSM) and chemical compositional analysis. Using these techniques we have studied carbonate sediment samples from Discovery Bay, Jamaica, which has been impacted to varying degrees by a bauxite loading facility. The carbonate sediment samples contain magnetic minerals ranging from moderate to low concentrations. The ESR spectra for all sites essentially contain three components. First, a six-line spectra centred around g = 2 resulting from Mn2+ ions within a carbonate matrix; second a g = 4.3 signal from isolated Fe3+ ions incorporated as impurities within minerals such as gibbsite, kaolinite or quartz; third a ferrimagnetic resonance with a maxima at 230 mT resulting from the ferrimagnetic minerals present within the bauxite contamination. Depending upon the location of the sites within the embayment these signals vary in their relative amplitude in a systematic manner related to the degree of bauxite input. Analysis of the ESR spectral components reveals linear relationships between the amplitude of the Mn2+ and ferrimagnetic signals and total Mn and Fe concentrations. To assist in determining the origin of the ESR signals coral and bauxite reference samples were employed. Coral representative of the matrix of the sediment was taken remote from the bauxite loading facility whilst pure bauxite was collected from nearby mining facilities. We find ESR to be a very sensitive technique particularly appropriate to magnetic analysis of ferri- and para-magnetic components within environmental samples otherwise dominated by diamagnetic (carbonate) minerals. When employing typical sample masses of 200 mg the practical detection limit of ESR to ferri- and para-magnetic minerals within a diamagnetic carbonate matrix is of the order of 1 ppm and 1 ppb

  17. A high sensitive 66 dB linear dynamic range receiver for 3-D laser radar

    Science.gov (United States)

    Ma, Rui; Zheng, Hao; Zhu, Zhangming

    2017-08-01

    This study presents a CMOS receiver chip realized in 0.18 μm standard CMOS technology and intended for high precision 3-D laser radar. The chip includes an adjustable gain transimpedance pre-amplifier, a post-amplifier and two timing comparators. An additional feedback is employed in the regulated cascode transimpedance amplifier to decrease the input impedance, and a variable gain transimpedance amplifier controlled by digital switches and analog multiplexer is utilized to realize four gain modes, extending the input dynamic range. The measurement shows that the highest transimpedance of the channel is 50 k {{Ω }}, the uncompensated walk error is 1.44 ns in a wide linear dynamic range of 66 dB (1:2000), and the input referred noise current is 2.3 pA/\\sqrt{{Hz}} (rms), resulting in a very low detectable input current of 1 μA with SNR = 5.

  18. Highly sensitive panchromatic ternary polymer photodetectors enabled by Förster resonance energy transfer and post solvent treatment

    Science.gov (United States)

    Wang, Hanyu; Zheng, Yifan; Qin, Ruiheng; Yu, Junsheng

    2018-03-01

    A panchromatic ternary polymer photodetector (PPD) with broadband response from 300 to 1000 nm is fabricated via incorporating poly({4,8-bis[(2-ethylhexyl)oxy]benzo[1,2-b:4,5-bʹ]dithiophene-2,6-diyl}{3-fluoro-2-[(2-ethylhexyl)carbonyl]thieno[3,4-b]thiophenediyl}) (PTB7) as the third component in poly(diketopyrrolopyrrole-terthiophene) (PDPP3T) [6]:-phenyl-C71-butyric acid methyl ester (PC71BM), revealing a high detectivity (D *) of 7.02  ×  1011 Jones at 850 nm. Through the analysis of photoluminescence and external quantum efficiency spectroscopy, we find that PTB7 can not only improve the absorption between 500-750 nm to induce more excitons, but also provide non-radiative transfer energy to PDPP3T via Förster resonance energy transfer (FRET). Moreover, we employ post solvent treatment (PST) to rectify the morphology of ternary blends, thus reducing charge recombination, suppressing dark current, and boosting the D * to 1.57  ×  1012 Jones at 850 nm, which is 2.34 folds higher than that of the untreated PPDs. This work indicates that the incorporation of FRET donor and PST in ternary blends is an effective way to develop highly sensitive panchromatic PPDs.

  19. High-sensitivity detection of polysaccharide using phosphodiesters quaternary ammonium salt as probe by decreased resonance light scattering.

    Science.gov (United States)

    Chen, Zhanguang; Liu, Guoliang; Chen, Maohuai; Wu, Mingyao

    2009-07-15

    Phosphodiesters quaternary ammonium salt (PQAS) displayed quite intense light scattering in aqueous solution under the optimum condition. In addition, the resonance light scattering (RLS) signal of PQAS was remarkably decreased after adding trace amount polysaccharide with the maximum peak located at 391 nm. It was found that the decreased RLS intensity of the PQAS-PPGL system (DeltaI(RLS)) was in proportion to PPGL concentration in the range of 0.1-30 ng mL(-1), with a lower detection limit of 0.05 ng mL(-1). Based on this rare decreased RLS phenomenon, the novel method of the determination of purified polysaccharide of Gracilaria Lemaneiformis (PPGL) at nanogram level was proposed in this contribution. The proposed approach was used to determine purified polysaccharide extracted from Gracilaria Lemaneiformis with satisfactory results. Compared with the reported polysaccharide assays, this proposed method has good selectivity, high sensitivity and is especially simple and convenient. Moreover, the mechanism of the reaction between PQAS and polysaccharide was investigated by RLS, fluorescence, and fluorescence lifetime spectra.

  20. Highly Sensitive Fluorescent Sensor for Cartap Based on Fluorescence Resonance Energy Transfer Between Gold Nanoparticles and Rhodamine B.

    Science.gov (United States)

    Dong, Liang; Hou, Changjun; Fa, Huanbao; Yang, Mei; Wu, Huixiang; Zhang, Liang; Huo, Danqun

    2018-04-01

    Cartap residue poses a great threat to human health and its derivatives would remain in soils, natural waters and other environmental domains for a long time. Herein, a simple, rapid and ultrasensitive analytical method for the determination of cartap based on fluorescence resonance energy transfer (FRET) between Au nanoparticles (AuNPs) and rhodamine B (RB) is first described. With the presence of citrate-stabilized AuNPs, the fluorescence of RB was remarkably quenched by AuNPs via FRET. The fluorescence of the AuNPs-RB system was recovered upon addition of cartap, cartap can be adsorbed on the surface of AuNPs due to its amino group that has good affinity with gold, which could induce the aggregation of AuNPs accompanying color change from red to blue. Thus, the FRET between AuNPs and RB was weakened and the PL intensity of RB was recovered accordingly. A good linear correlation for detection of RB was exhibited from 1 nM to 180 nM, and the detection limit reached 0.88 nM, which was much lower than the safety limit required by USA, UK and China. To the best of our knowledge, it has been the lowest detection ever without the aid of costly instrumentation. This method was successfully carried out for the assessment of cartap in real samples with satisfactory results, which revealed many advantages such as high sensitivity, low cost and non-time-consuming compared with traditional methods.

  1. High Temperature and High Sensitive NOx Gas Sensor with Hetero-Junction Structure using Laser Ablation Method

    Science.gov (United States)

    Gao, Wei; Shi, Liqin; Hasegawa, Yuki; Katsube, Teruaki

    In order to develop a high temperature (200°C˜400°C) and high sensitive NOx gas sensor, we developed a new structure of SiC-based hetero-junction device Pt/SnO2/SiC/Ni, Pt/In2O3/SiC/Ni and Pt/WO3/SiC/Ni using a laser ablation method for the preparation of both metal (Pt) electrode and metal-oxide film. It was found that Pt/In2O3/SiC/Ni sensor shows higher sensitivity to NO2 gas compared with the Pt/SnO2/SiC/Ni and Pt/WO3/SiC/Ni sensor, whereas the Pt/WO3/SiC/Ni sensor had better sensitivity to NO gas. These results suggest that selective detection of NO and NO2 gases may be obtained by choosing different metal oxide films.

  2. Highly sensitive and selective cartap nanosensor based on luminescence resonance energy transfer between NaYF4:Yb,Ho nanocrystals and gold nanoparticles.

    Science.gov (United States)

    Wang, Zhijiang; Wu, Lina; Shen, Baozhong; Jiang, Zhaohua

    2013-09-30

    Fluorescent detection is an attractive method for the detection of toxic chemicals. However, most chemosensors that are currently utilized in fluorescent detection are based on organic dyes or quantum dots, which suffer from instability, high background noise and interference from organic impurities in solution, which can also be excited by UV radiation. In the present research, we developed a novel NaYF4:Yb,Ho/Au nanocomposite-based chemosensor with high sensitivity (10 ppb) and selectivity over competing analytes for the detection of the insecticide cartap. This nanosensor is excited with a 970-nm laser instead of UV radiation to give an emission peak at 541 nm. In the presence of cartap, the nanocomposites aggregate, resulting in enhanced luminescence resonance energy transfer between the NaYF4:Yb,Ho nanocrystals and the gold nanoparticles, which decreases the emission intensity at 541 nm. The relative luminescence intensity at 541 nm has a linear relationship with the concentration of cartap in the solution. Based on this behavior, the developed nanosensor successfully detected cartap in farm produce and water samples with satisfactory results. Copyright © 2013 Elsevier B.V. All rights reserved.

  3. Highly sensitive and selective determination of hydrogen sulfide by resonance light scattering technique based on silver nanoparticles.

    Science.gov (United States)

    Kuang, Yangfang; Chen, Shu; Long, Yunfei

    2017-06-01

    We have developed a green approach to prepare DNA-templated silver nanoparticles (Ag-NPs) from the direct reaction between Ag + and ascorbic acid in the presence of DNA and sodium hydroxide. The Ag-NPs showed strong resonance light scattering (RLS) intensity property. Then, the interaction between hydrogen sulfide (H 2 S) and Ag-NPs was studied by measuring their RLS spectra. The results showed that there is a strong interaction between Ag-NPs and H 2 S, which resulted in a decrease in the size of Ag-NPs and a decrease in the RLS intensity of the Ag-NPs solution at the wavelength of 467 nm. The results demonstrated that the RLS technique offers a sensitive and simple tool for investigating the interaction between Ag-NPs and H 2 S, which can be applied to detect H 2 S with high sensitivity and selectivity without complex readout equipment. The linear range for H 2 S determination was found to be the range from 5.0 × 10 -9 to 1.0 × 10 -7  mol L -1 , and the detection limit (3σ/k) was 2.8 × 10 -9  mol L -1 . Moreover, the proposed method was applied for the determination of H 2 S in natural water samples with satisfactory results. Graphical abstract The application of Ag-NPs in H 2 S detection.

  4. Numerical simulation of laser resonators

    International Nuclear Information System (INIS)

    Yoo, J. G.; Jeong, Y. U.; Lee, B. C.; Rhee, Y. J.; Cho, S. O.

    2004-01-01

    We developed numerical simulation packages for laser resonators on the bases of a pair of integral equations. Two numerical schemes, a matrix formalism and an iterative method, were programmed for finding numeric solutions to the pair of integral equations. The iterative method was tried by Fox and Li, but it was not applicable for high Fresnel numbers since the numerical errors involved propagate and accumulate uncontrollably. In this paper, we implement the matrix method to extend the computational limit further. A great number of case studies are carried out with various configurations of stable and unstable r;esonators to compute diffraction losses, phase shifts, intensity distributions and phases of the radiation fields on mirrors. Our results presented in this paper show not only a good agreement with the results previously obtained by Fox and Li, but also the legitimacy of our numerical procedures for high Fresnel numbers.

  5. Widely tunable asymmetric long-period fiber grating with high sensitivity using optical polymer on laser-ablated cladding.

    Science.gov (United States)

    Chen, Nan-Kuang; Hsu, Der-Yi; Chi, Sien

    2007-08-01

    We demonstrate high-efficiency, wideband-tunable, laser-ablated long-period fiber gratings that use an optical polymer overlay. Portions of the fiber cladding are periodically removed by CO(2) laser pulses to induce periodic index changes for coupling the core mode into cladding modes. An optical polymer with a high thermo-optic coefficient with a dispersion distinct from that of silica is used on a deep-ablated cladding structure so that the effective indices of cladding modes become dispersive and the resonant wavelengths can be efficiently tuned. The tuning efficiency can be as high as 15.8 nm/ degrees C, and the tuning range can be wider than 105 nm (1545-1650 nm).

  6. High-Sensitivity Spectrophotometry.

    Science.gov (United States)

    Harris, T. D.

    1982-01-01

    Selected high-sensitivity spectrophotometric methods are examined, and comparisons are made of their relative strengths and weaknesses and the circumstances for which each can best be applied. Methods include long path cells, noise reduction, laser intracavity absorption, thermocouple calorimetry, photoacoustic methods, and thermo-optical methods.…

  7. Electromechanical model of a resonating nano-cantilever-based sensor for high-resolution and high-sensitivity mass detection

    DEFF Research Database (Denmark)

    Abadal, G.; Davis, Zachary James; Helbo, Bjarne

    2001-01-01

    A simple linear electromechanical model for an electrostatically driven resonating cantilever is derived. The model has been developed in order to determine dynamic quantities such as the capacitive current flowing through the cantilever-driver system at the resonance frequency, and it allows us ...

  8. Development of a high-sensitivity and portable cell using Helmholtz resonance for noninvasive blood glucose-level measurement based on photoacoustic spectroscopy.

    Science.gov (United States)

    Tachibana, K; Okada, K; Kobayashi, R; Ishihara, Y

    2016-08-01

    We describe the possibility of high-sensitivity noninvasive blood glucose measurement based on photoacoustic spectroscopy (PAS). The demand for noninvasive blood glucose-level measurement has increased due to the explosive increase in diabetic patients. We have developed a noninvasive blood glucose-level measurement based on PAS. The conventional method uses a straight-type resonant cell. However, the cell volume is large, which results in a low detection sensitivity and difficult portability. In this paper, a small-sized Helmholtz-type resonant cell is proposed to improve detection sensitivity and portability by reducing the cell dead volume. First, the acoustic property of the small-sized Helmholtz-type resonant cell was evaluated by performing an experiment using a silicone rubber. As a result, the detection sensitivity of the small-sized Helmholtz-type resonant cell was approximately two times larger than that of the conventional straight-type resonant cell. In addition, the inside volume was approximately 30 times smaller. Second, the detection limits of glucose concentration were estimated by performing an experiment using glucose solutions. The experimental results showed that a glucose concentration of approximately 1% was detected by the small-sized Helmholtz-type resonant cell. Although these results on the sensitivity of blood glucose-level measurement are currently insufficient, they suggest that miniaturization of a resonance cell is effective in the application of noninvasive blood glucose-level measurement.

  9. Coupled optical resonance laser locking.

    Science.gov (United States)

    Burd, S C; du Toit, P J W; Uys, H

    2014-10-20

    We have demonstrated simultaneous laser frequency stabilization of a UV and IR laser, to coupled transitions of ions in the same spectroscopic sample, by detecting only the absorption of the UV laser. Separate signals for locking the different lasers are obtained by modulating each laser at a different frequency and using lock-in detection of a single photodiode signal. Experimentally, we simultaneously lock a 369 nm and a 935 nm laser to the (2)S(1/2) → (2)(P(1/2) and (2)D(3/2) → (3)D([3/2]1/2) transitions, respectively, of Yb(+) ions generated in a hollow cathode discharge lamp. Stabilized lasers at these frequencies are required for cooling and trapping Yb(+) ions, used in quantum information and in high precision metrology experiments. This technique should be readily applicable to other ion and neutral atom systems requiring multiple stabilized lasers.

  10. High frame rate multi-resonance imaging refractometry with distributed feedback dye laser sensor

    DEFF Research Database (Denmark)

    Vannahme, Christoph; Dufva, Martin; Kristensen, Anders

    2015-01-01

    imaging refractometry without moving parts is presented. DFB dye lasers are low-cost and highly sensitive refractive index sensors. The unique multi-wavelength DFB laser structure presented here comprises several areas with different grating periods. Imaging in two dimensions of space is enabled...... by analyzing laser light from all areas in parallel with an imaging spectrometer. With this multi-resonance imaging refractometry method, the spatial position in one direction is identified from the horizontal, i.e., spectral position of the multiple laser lines which is obtained from the spectrometer charged...

  11. Coupled optical resonance laser locking

    CSIR Research Space (South Africa)

    Burd, CC

    2014-10-01

    Full Text Available We have demonstrated simultaneous laser frequency stabilization of a UV and IR laser, to coupled transitions of ions in the same spectroscopic sample, by detecting only the absorption of the UV laser. Separate signals for locking the different...

  12. Laser resonant ionization spectroscopy and laser-induced resonant fluorescence spectra of samarium atom

    International Nuclear Information System (INIS)

    Jin, Changtai

    1995-01-01

    We have measured new high-lying levels of Sm atom by two-colour resonant photoionisation spectroscopy; we have observed the isotope shifts of Sm atom by laser-induced resonant fluorescence spectroscopy; the lifetime of eight low-lying levels of Sm atom were measured by using pulsed laser-Boxcar technique in atomic beam.

  13. Monolithic optofluidic ring resonator lasers created by femtosecond laser nanofabrication.

    Science.gov (United States)

    Chandrahalim, Hengky; Chen, Qiushu; Said, Ali A; Dugan, Mark; Fan, Xudong

    2015-05-21

    We designed, fabricated, and characterized a monolithically integrated optofluidic ring resonator laser that is mechanically, thermally, and chemically robust. The entire device, including the ring resonator channel and sample delivery microfluidics, was created in a block of fused-silica glass using a 3-dimensional femtosecond laser writing process. The gain medium, composed of Rhodamine 6G (R6G) dissolved in quinoline, was flowed through the ring resonator. Lasing was achieved at a pump threshold of approximately 15 μJ mm(-2). Detailed analysis shows that the Q-factor of the optofluidic ring resonator is 3.3 × 10(4), which is limited by both solvent absorption and scattering loss. In particular, a Q-factor resulting from the scattering loss can be as high as 4.2 × 10(4), suggesting the feasibility of using a femtosecond laser to create high quality optical cavities.

  14. Limited magnetic resonance imaging of the lumbar spine has high sensitivity for detection of acute fractures, infection, and malignancy

    International Nuclear Information System (INIS)

    Wang, Benjamin; Fintelmann, Florian J.; Kamath, Ravi S.; Kattapuram, Susan V.; Rosenthal, Daniel I.

    2016-01-01

    The objective of this study is to determine how a limited protocol MR examination compares to a full conventional MR examination for the detection of non-degenerative pathology such as acute fracture, infection, and malignancy. A sample of 349 non-contrast MR exams was selected retrospectively containing a 3:1:1:1 distribution of negative/degenerative change only, acute fracture, infection, and malignancy. This resulted in an even distribution of pathology and non-pathology. A limited protocol MR exam was simulated by extracting T1-weighted sagittal and T2-weighted fat-saturated (or STIR) sagittal sequences from each exam and submitting them for blinded review by two experienced musculoskeletal radiologists. The exams were evaluated for the presence or absence of non-degenerative pathology. Interpretation of the limited exam was compared to the original report of the full examination. If either reader disagreed with the original report, the case was submitted for an unblinded adjudication process with the participation of a third musculoskeletal radiologist to establish a consensus diagnosis. There were five false negatives for a sensitivity of 96.9 % for the limited protocol MR exam. Infection in the psoas, paraspinal muscles, and sacroiliac joint, as well as acute fractures in transverse processes and sacrum were missed by one or more readers. No cases of malignancy were missed. Overall diagnostic accuracy was 96.0 % (335/349). MR imaging of the lumbar spine limited to sagittal T1-weighted and sagittal T2 fat-saturated (or STIR) sequences has high sensitivity for the detection of acute fracture, infection, or malignancy compared to a conventional MR examination. (orig.)

  15. Limited magnetic resonance imaging of the lumbar spine has high sensitivity for detection of acute fractures, infection, and malignancy

    Energy Technology Data Exchange (ETDEWEB)

    Wang, Benjamin; Fintelmann, Florian J.; Kamath, Ravi S.; Kattapuram, Susan V.; Rosenthal, Daniel I. [Massachusetts General Hospital, Department of Radiology, Boston, MA (United States)

    2016-12-15

    The objective of this study is to determine how a limited protocol MR examination compares to a full conventional MR examination for the detection of non-degenerative pathology such as acute fracture, infection, and malignancy. A sample of 349 non-contrast MR exams was selected retrospectively containing a 3:1:1:1 distribution of negative/degenerative change only, acute fracture, infection, and malignancy. This resulted in an even distribution of pathology and non-pathology. A limited protocol MR exam was simulated by extracting T1-weighted sagittal and T2-weighted fat-saturated (or STIR) sagittal sequences from each exam and submitting them for blinded review by two experienced musculoskeletal radiologists. The exams were evaluated for the presence or absence of non-degenerative pathology. Interpretation of the limited exam was compared to the original report of the full examination. If either reader disagreed with the original report, the case was submitted for an unblinded adjudication process with the participation of a third musculoskeletal radiologist to establish a consensus diagnosis. There were five false negatives for a sensitivity of 96.9 % for the limited protocol MR exam. Infection in the psoas, paraspinal muscles, and sacroiliac joint, as well as acute fractures in transverse processes and sacrum were missed by one or more readers. No cases of malignancy were missed. Overall diagnostic accuracy was 96.0 % (335/349). MR imaging of the lumbar spine limited to sagittal T1-weighted and sagittal T2 fat-saturated (or STIR) sequences has high sensitivity for the detection of acute fracture, infection, or malignancy compared to a conventional MR examination. (orig.)

  16. A reduced graphene oxide-based fluorescence resonance energy transfer sensor for highly sensitive detection of matrix metalloproteinase 2.

    Science.gov (United States)

    Xi, Gaina; Wang, Xiaoping; Chen, Tongsheng

    2016-01-01

    A novel fluorescence nanoprobe (reduced nano-graphene oxide [nrGO]/fluorescein isothiocyanate-labeled peptide [Pep-FITC]) for ultrasensitive detection of matrix metalloproteinase 2 (MMP2) has been developed by engineering the Pep-FITC comprising the specific MMP2 substrate domain (PLGVR) onto the surface of nrGO particles through non-covalent linkage. The nrGO was obtained by water bathing nano-graphene oxide under 90°C for 4 hours. After mixing the nrGO and Pep-FITC for 30 seconds, the fluorescence from Pep-FITC was almost completely quenched due to the fluorescence resonance energy transfer between fluorescein isothiocyanate (FITC) and nrGO. Upon cleavage of the amide bond between Leu and Gly in the Pep-FITC by protease-MMP2, the FITC bound to nrGO was separated from nrGO surface, disrupting the fluorescence resonance energy transfer process and resulting in fluorescence recovery of FITC. Under optimal conditions, the fluorescence recovery of nrGO/Pep-FITC was found to be directly proportional to the concentration of MMP2 within 0.02-0.1 nM. The detection limit of the nrGO/Pep-FITC was determined to be 3 pM, which is approximately tenfold lower than that of the unreduced carboxylated nano-graphene oxide/Pep-FITC probe.

  17. High sensitive detection of copper II ions using D-penicillamine-coated gold nanorods based on localized surface plasmon resonance

    Science.gov (United States)

    Hong, Yoochan; Jo, Seongjae; Park, Joohyung; Park, Jinsung; Yang, Jaemoon

    2018-05-01

    In this paper, we describe the development of a nanoplasmonic biosensor based on the localized surface plasmon resonance (LSPR) effect that enables a sensitive and selective recognition of copper II ions. First, we fabricated the nanoplasmonics as LSPR substrates using gold nanorods (GNR) and the nano-adsorption method. The LSPR sensitivity of the nanoplasmonics was evaluated using various solvents with different refractive indexes. Subsequently, D-penicillamine (DPA)—a chelating agent of copper II ions—was conjugated to the surface of the GNR. The limit of detection (LOD) for the DPA-conjugated nanoplasmonics was 100 pM. Furthermore, selectivity tests were conducted using various divalent cations, and sensitivity tests were conducted on the nanoplasmonics under blood-like environments. Finally, the developed nanoplasmonic biosensor based on GNR shows great potential for the effective recognition of copper II ions, even in human blood conditions.

  18. Unstable Resonator Retrofitted Handheld Laser Designator

    Science.gov (United States)

    1978-06-01

    retrofitted with a negative-branch unstable resona- tor laser and hybrid pump cavity in place of the conventional plane-mirror/ porro prism resonator and...directed by prism B to an expanding telescope, shared with the viewing system of the designator. The actual, unfolded resonator length is approxi...was performed based on using a plane- parallel cavity consisting of a 47% reflectivity output coupler, porro - prism reflector, and the same LiNb03

  19. Highly sensitive analysis of boron and lithium in aqueous solution using dual-pulse laser-induced breakdown spectroscopy.

    Science.gov (United States)

    Lee, Dong-Hyoung; Han, Sol-Chan; Kim, Tae-Hyeong; Yun, Jong-Il

    2011-12-15

    We have applied a dual-pulse laser-induced breakdown spectroscopy (DP-LIBS) to sensitively detect concentrations of boron and lithium in aqueous solution. Sequential laser pulses from two separate Q-switched Nd:YAG lasers at 532 nm wavelength have been employed to generate laser-induced plasma on a water jet. For achieving sensitive elemental detection, the optimal timing between two laser pulses was investigated. The optimum time delay between two laser pulses for the B atomic emission lines was found to be less than 3 μs and approximately 10 μs for the Li atomic emission line. Under these optimized conditions, the detection limit was attained in the range of 0.8 ppm for boron and 0.8 ppb for lithium. In particular, the sensitivity for detecting boron by excitation of laminar liquid jet was found to be excellent by nearly 2 orders of magnitude compared with 80 ppm reported in the literature. These sensitivities of laser-induced breakdown spectroscopy are very practical for the online elemental analysis of boric acid and lithium hydroxide serving as neutron absorber and pH controller in the primary coolant water of pressurized water reactors, respectively.

  20. Investigation of ultra-high sensitivity Klystron cavity transducers for broadband resonant-mass gravitational wave detectors

    International Nuclear Information System (INIS)

    Pimentel, Guilherme Leite

    2008-01-01

    We show that, with a suitable choice of the parameters of the gravitational wave detector Mario Schoenberg, with technological accessible parameters (using state-of-art electronics), its sensitivity curve can be improved over the current project curve to become competitive with interferometric detectors in a frequency band of 1500 Hz, in the region from 1000 to 10000 Hz (these competitive bands are centered at the sphere's quadrupole modes). The sensitivity curve of an array of 100 identical spheres identical to the Schoenberg one is also analyzed, and is competitive against advanced LIGO in the entire band. A detailed study of the project's viability is conducted, with an emphasis on the project of the klystron resonant cavity, which will have a center post with a 1 nm gap, which represents a great technological challenge. This challenge is analyzed in terms of the cavity project as well as with a focus on the Casimir effect on the cavity. This could open an opportunity for precise measurements of this effect on a new distance scale compared to current measurements (in the μm scale). (author)

  1. Development of high sensitivity eight-element multiplexed fiber laser acoustic pressure hydrophone array and interrogation system

    Science.gov (United States)

    Li, Ming; Sun, Zhihui; Zhang, Xiaolei; Li, Shujuan; Song, Zhiqiang; Wang, Meng; Guo, Jian; Ni, Jiasheng; Wang, Chang; Peng, Gangding; Xu, Xiangang

    2017-09-01

    Fiber laser hydrophones have got widespread concerns due to the unique advantages and broad application prospects. In this paper, the research results of the eight-element multiplexed fiber laser acoustic pressure array and the interrogation system are introduced, containing low-noise distributed feedback fiber laser (DFB-FL) fabrication, sensitivity enhancement packaging, and interferometric signal demodulation. The frequency response range of the system is 10Hz-10kHz, the laser frequency acoustic pressure sensitivity reaches 115 dB re Hz/Pa, and the equivalent noise acoustic pressure is less than 60μPa/Hz1/2. The dynamic range of the system is greater than 120 dB.

  2. High sensitivity detection of NO2 employing cavity ringdown spectroscopy and an external cavity continuously tunable quantum cascade laser.

    Science.gov (United States)

    Rao, Gottipaty N; Karpf, Andreas

    2010-09-10

    A trace gas sensor for the detection of nitrogen dioxide based on cavity ringdown spectroscopy (CRDS) and a continuous wave external cavity tunable quantum cascade laser operating at room temperature has been designed, and its features and performance characteristics are reported. By measuring the ringdown times of the cavity at different concentrations of NO(2), we report a sensitivity of 1.2 ppb for the detection of NO(2) in Zero Air.

  3. Graphene functionalised by laser-ablated V2O5 for a highly sensitive NH3 sensor

    Directory of Open Access Journals (Sweden)

    Margus Kodu

    2017-03-01

    Full Text Available Graphene has been recognized as a promising gas sensing material. The response of graphene-based sensors can be radically improved by introducing defects in graphene using, for example, metal or metal oxide nanoparticles. We have functionalised CVD grown, single-layer graphene by applying pulsed laser deposition (PLD of V2O5 which resulted in a thin V2O5 layer on graphene with average thickness of ≈0.6 nm. From Raman spectroscopy, it was concluded that the PLD process also induced defects in graphene. Compared to unmodified graphene, the obtained chemiresistive sensor showed considerable improvement of sensing ammonia at room temperature. In addition, the response time, sensitivity and reversibility were essentially enhanced due to graphene functionalisation by laser deposited V2O5. This can be explained by an increased surface density of gas adsorption sites introduced by high energy atoms in laser ablation plasma and formation of nanophase boundaries between deposited V2O5 and graphene.

  4. Cyclotron resonance cooling by strong laser field

    International Nuclear Information System (INIS)

    Tagcuhi, Toshihiro; Mima, Kunioka

    1995-01-01

    Reduction of energy spread of electron beam is very important to increase a total output radiation power in free electron lasers. Although several cooling systems of particle beams such as a stochastic cooling are successfully operated in the accelerator physics, these cooling mechanisms are very slow and they are only applicable to high energy charged particle beams of ring accelerators. We propose here a new concept of laser cooling system by means of cyclotron resonance. Electrons being in cyclotron motion under a strong magnetic field can resonate with circular polarized electromagnetic field, and the resonance take place selectively depending on the velocity of the electrons. If cyclotron frequency of electrons is equal to the frequency of the electromagnetic field, they absorb the electromagnetic field energy strongly, but the other electrons remain unchanged. The absorbed energy will be converted to transverse kinetic energy, and the energy will be dumped into the radiation energy through bremastrahlung. To build a cooling system, we must use two laser beams, where one of them is counter-propagating and the other is co-propagating with electron beam. When the frequency of the counter-propagating laser is tuned with the cyclotron frequency of fast electrons and the co-propagating laser is tuned with the cyclotron frequency of slow electrons, the energy of two groups will approach and the cooling will be achieved. We solve relativistic motions of electrons with relativistic radiation dumping force, and estimate the cooling rate of this mechanism. We will report optimum parameters for the electron beam cooling system for free electron lasers

  5. A Q-switched Ho:YAG laser assisted nanosecond time-resolved T-jump transient mid-IR absorbance spectroscopy with high sensitivity

    Energy Technology Data Exchange (ETDEWEB)

    Li, Deyong; Li, Yunliang; Li, Hao; Weng, Yuxiang, E-mail: yxweng@iphy.ac.cn [Key Laboratory of Soft Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China); Wu, Xianyou [Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031 (China); Yu, Qingxu [School of Physics and Optoelectronic Technology, Dalian University of Technology, No. 2, Linggong Road, Dalian 116023 (China)

    2015-05-15

    Knowledge of dynamical structure of protein is an important clue to understand its biological function in vivo. Temperature-jump (T-jump) time-resolved transient mid-IR absorbance spectroscopy is a powerful tool in elucidating the protein dynamical structures and the folding/unfolding kinetics of proteins in solution. A home-built setup of T-jump time-resolved transient mid-IR absorbance spectroscopy with high sensitivity is developed, which is composed of a Q-switched Cr, Tm, Ho:YAG laser with an output wavelength at 2.09 μm as the T-jump heating source, and a continuous working CO laser tunable from 1580 to 1980 cm{sup −1} as the IR probe. The results demonstrate that this system has a sensitivity of 1 × 10{sup −4} ΔOD for a single wavelength detection, and 2 × 10{sup −4} ΔOD for spectral detection in amide I′ region, as well as a temporal resolution of 20 ns. Moreover, the data quality coming from the CO laser is comparable to the one using the commercial quantum cascade laser.

  6. Resonant Laser Manipulation of an Atomic Beam

    Science.gov (United States)

    2010-07-01

    Technical Paper 3. DATES COVERED (From - To) 4. TITLE AND SUBTITLE 5a. CONTRACT NUMBER Resonant Laser Manipulation of an Atomic Beam...steering and collimating flows with higher densities and energies than current common practice . One impediment to this extension is the development of...where Δεg is the ground state Stark shift, Ω is the Rabi frequency (related to intensity), Isat is the saturation intensity of the transition, and I(r

  7. Resonance Rayleigh Scattering Spectra of an Ion-Association Complex of Naphthol Green B–Chitosan System and Its Application in the Highly Sensitive Determination of Chitosan

    Directory of Open Access Journals (Sweden)

    Weiai Zhang

    2016-04-01

    Full Text Available This work describes a highly-sensitive and accurate approach for the determination of chitosan (CTS using Naphthol Green B (NGB as a probe in the Resonance Rayleigh scattering (RRS method. The interaction between CTS and NGB leads to notable enhancement of RRS, and the enhancement is proportional to the concentration of CTS over a certain range. Under optimum conditions, the calibration curve of ΔI against CTS concentration was ΔI = 1860.5c + 86.125 (c, µg/mL, R2 = 0.9999, and the linear range and detection limit (DL were 0.01–5.5 µg/mL and 8.87 ng/mL. Moreover, the effect of the molecular weight of CTS on the accurate quantification of CTS was studied. The experimental data were analyzed through linear regression analysis using SPSS20.0, and the molecular weight was found to have no statistical significance. This method has been applied to assay two CTS samples and obtained good recovery and reproducibility.

  8. Superthin resonator dye laser with THz intermode frequency separation

    International Nuclear Information System (INIS)

    Rudych, P D; Surovtsev, N V

    2014-01-01

    Two-color laser irradiation is considered an effective way to pump THz excitations for numerous scientific and applied goals. We present a design for convenient laser source with THz intermode frequency separation. The setup is based on dye laser with superthin resonator pumped by a subnanosecond pulse laser. It was proven that the superthin resonator dye laser is useful, possesses high stability and high energy conversion, and generates narrow laser modes. The ability of this laser to pump CARS processes for THz vibrations is demonstrated. (letter)

  9. Rapid, simple, and highly sensitive analysis of drugs in biological samples using thin-layer chromatography coupled with matrix-assisted laser desorption/ionization mass spectrometry.

    Science.gov (United States)

    Kuwayama, Kenji; Tsujikawa, Kenji; Miyaguchi, Hajime; Kanamori, Tatsuyuki; Iwata, Yuko T; Inoue, Hiroyuki

    2012-01-01

    Rapid and precise identification of toxic substances is necessary for urgent diagnosis and treatment of poisoning cases and for establishing the cause of death in postmortem examinations. However, identification of compounds in biological samples using gas chromatography and liquid chromatography coupled with mass spectrometry entails time-consuming and labor-intensive sample preparations. In this study, we examined a simple preparation and highly sensitive analysis of drugs in biological samples such as urine, plasma, and organs using thin-layer chromatography coupled with matrix-assisted laser desorption/ionization mass spectrometry (TLC/MALDI/MS). When the urine containing 3,4-methylenedioxymethamphetamine (MDMA) without sample dilution was spotted on a thin-layer chromatography (TLC) plate and was analyzed by TLC/MALDI/MS, the detection limit of the MDMA spot was 0.05 ng/spot. The value was the same as that in aqueous solution spotted on a stainless steel plate. All the 11 psychotropic compounds tested (MDMA, 4-hydroxy-3-methoxymethamphetamine, 3,4-methylenedioxyamphetamine, methamphetamine, p-hydroxymethamphetamine, amphetamine, ketamine, caffeine, chlorpromazine, triazolam, and morphine) on a TLC plate were detected at levels of 0.05-5 ng, and the type (layer thickness and fluorescence) of TLC plate did not affect detection sensitivity. In addition, when rat liver homogenate obtained after MDMA administration (10 mg/kg) was spotted on a TLC plate, MDMA and its main metabolites were identified using TLC/MALDI/MS, and the spots on a TLC plate were visualized by MALDI/imaging MS. The total analytical time from spotting of intact biological samples to the output of analytical results was within 30 min. TLC/MALDI/MS enabled rapid, simple, and highly sensitive analysis of drugs from intact biological samples and crude extracts. Accordingly, this method could be applied to rapid drug screening and precise identification of toxic substances in poisoning cases and

  10. Bullet Design and Fabrication of Dual Mode Pyroelectric Sensor: High Sensitive Energymeter for Nd: YAG Laser and Detector for Chopped He-Ne Laser

    Directory of Open Access Journals (Sweden)

    S. SATAPATHY

    2008-05-01

    Full Text Available Pyroelectric sensor using TGS has been designed and fabricated which can be operated in laser energy meter mode as well as pyroelectric detector mode. The amplifying circuit configuration has very good signal to noise ratio, very high input impedance and low drift. The pyroelectric sensor has been tested using Q-switched Nd: YAG laser and chopped He-Ne laser. The sensitivity of pyroelectric sensor in energymeter mode is 421.7V/J and the voltage responsivity of the pyroelectric sensor is 3.27 V/W in detector mode.

  11. Stimulated resonance Raman spectroscopy: An alternative to laser-rf double resonance for ion spectroscopy

    International Nuclear Information System (INIS)

    Young, L.; Dinneen, T.; Mansour, N.B.

    1988-01-01

    Stimulated resonance Raman spectroscopy is presented as an alternative to laser-rf double resonance for obtaining high-precision measurements in ion beams. By use of a single-phase modulated laser beam to derive the two required fields, the laser--ion-beam alignment is significantly simplified. In addition, this method is especially useful in the low-frequency regime where the laser-rf double-resonance method encounters difficulties due to modifications of the ion-beam velocity distribution. These modifications, which result from interaction with the traveling rf wave used to induce magnetic dipole transitions, are observed and quantitatively modeled

  12. Spontaneous generation of vortex and coherent vector beams from a thin-slice c-cut Nd:GdVO4 laser with wide-aperture laser-diode end pumping: application to highly sensitive rotational and translational Doppler velocimetry

    Science.gov (United States)

    Otsuka, Kenju; Chu, Shu-Chun

    2017-07-01

    Selective excitation of Laguerre-Gauss modes (optical vortices: helical LG0,2 and LG0,1), reflecting their weak transverse cross-saturation of population inversions against a preceding higher-order Ince-Gauss (IG0,2) or Hermite-Gauss (HG2,1) mode, was observed in a thin-slice c-cut Nd:GdVO4 laser with wide-aperture laser-diode end pumping. Single-frequency coherent vector beams were generated through the transverse mode locking of a pair of orthogonally polarized IG2,0 and LG0,2 or HG2,1 and LG0,1 modes. Highly sensitive self-mixing rotational and translational Doppler velocimetry is demonstrated by using vortex and coherent vector beams.

  13. Resonance ionization spectroscopy using ultraviolet laser

    CERN Document Server

    Han, J M; Ko, D K; Park, H M; Rhee, Y J

    2002-01-01

    In this study, Ti:sapphire laser which is pumped by the enhanced Nd:YAG laser using laser diode, was designed and manufactured. The AO Q-switched CW Nd:YAG laser was converted into a high repetition plus-type laser using the AO Q-switch, and two heads were installed inside the cavity in order to improve the laser beam quality. The Nd:YAG laser enhancement was completed by optimization using a simulation for the cavity length, structure and thermal lens effect that greatly effected the laser beam output and quality. As the result of the enhancement, a 30W laser at 532nm and at 5k-Hz was successfully made. Also, the Ti:sapphire laser that will be used for atomic spectroscopy which is pumped by the Nd:YAG laser, was completely designed. As a basic experiment for laser oscillation. We measured the tunability of the laser, and it turned out that the wave tunability range was 730 850 nm. A self-seeding type tunable laser using grating for narrow line width, is planned to be designed due to the fact that the Ti:sapp...

  14. Experiments on resonantly photo-pumped x-ray lasers

    International Nuclear Information System (INIS)

    Nilsen, J.; Porter, J.L.; Da Silva, L.B.; MacGowan, B.; Beiersdorfer, P..; Elliott, S.R.; Young, B.K.

    1992-01-01

    We describe our recent effort to identify and study a promising resonantly photopumped x-ray laser scheme. In particular we will describe a scheme which uses the strong emission lines of a nickel-like ion to resonantly photo-pump a neon-like ion and enhance the lasing of the neon-like 3p → 3s transitions

  15. Laser modes and threshold condition i N-mirror resonator

    DEFF Research Database (Denmark)

    Pedersen, Christian; Skettrup, Torben

    1996-01-01

    Two formal methods for finding laser modes and threshold conditions in laser resonators containing as many as N mirrors are presented. The first method is based on an analysis determining the reflectivity and the transmittivity of an N-mirror system with gain. This is an extension of the classical...... 2 × 2 matrix method. The second method is based on self-consistency equations for the system and directly yields the circulating fields of the individual resonators. A set of rules has been proved to allow these fields to be calculated directly by means of inspection. The laser oscillation condition...

  16. Highly Sensitive Optical Receivers

    CERN Document Server

    Schneider, Kerstin

    2006-01-01

    Highly Sensitive Optical Receivers primarily treats the circuit design of optical receivers with external photodiodes. Continuous-mode and burst-mode receivers are compared. The monograph first summarizes the basics of III/V photodetectors, transistor and noise models, bit-error rate, sensitivity and analog circuit design, thus enabling readers to understand the circuits described in the main part of the book. In order to cover the topic comprehensively, detailed descriptions of receivers for optical data communication in general and, in particular, optical burst-mode receivers in deep-sub-µm CMOS are presented. Numerous detailed and elaborate illustrations facilitate better understanding.

  17. Resonance ionization mass spectrometry using tunable diode lasers

    International Nuclear Information System (INIS)

    Shaw, R.W.; Young, J.P.; Smith, D.H.

    1990-01-01

    Tunable semiconductor diode lasers will find many important applications in atomic spectroscopy. They exhibit the desirable attributes of lasers: narrow bandwidth, tunability, and spatial coherence. At the same time, they possess few of the disadvantages of other tunable lasers. They require no alignment, are simple to operate, and are inexpensive. Practical laser spectroscopic instruments can be envisioned. The authors have applied diode lasers to resonance ionization mass spectrometry (RIMS) of some of the lanthanide elements. Sub-Doppler resolution spectra have been recorded and have been used for atomic hyperfine structure analysis. Isotopically-selective ionization has been accomplished, even in cases where photons from a broadband dye laser are part of the overall ionization process and where the isotopic spectral shift is very small. A convenient RIMS instrument for isotope ratio measurements that employs only diode lasers, along with electric field ionization, should be possible

  18. Highly sensitive digital optical sensor with large measurement range based on the dual-microring resonator with waveguide-coupled feedback

    International Nuclear Information System (INIS)

    Xiang Xing-Ye; Wang Kui-Ru; Yuan Jin-Hui; Jin Bo-Yuan; Sang Xin-Zhu; Yu Chong-Xiu

    2014-01-01

    We propose a novel high-performance digital optical sensor based on the Mach—Zehnder interferential effect and the dual-microring resonators with the waveguide-coupled feedback. The simulation results show that the sensitivity of the sensor can be orders of magnitude higher than that of a conventional sensor, and high quality factor is not critical in it. Moreover, by optimizing the length of the feedback waveguide to be equal to the perimeter of the ring, the measurement range of the proposed sensor is twice as much as that of the conventional sensor in the weak coupling case

  19. Laser Resonators and Beam Propagation Fundamentals, Advanced Concepts and Applications

    CERN Document Server

    Hodgson, Norman

    2005-01-01

    Optical Resonators provides a detailed discussion of the properties of optical resonators for lasers from basic theory to recent research. In addition to describing the fundamental theories of resonators such as geometrical optics, diffraction, and polarisation the characteristics of all important resonator schemes and their calculation are presented. Experimental examples, practical problems and a collection of measurement techniques support the comprehensive treatment of the subject. Optical Resonators is the only book currently available that provides a comprehensive overview of the the subject. Combined with the structure of the text and the autonomous nature of the chapters this work will be as suitable for those new to the field as it will be invaluable to specialists conducting research. This second edition has been enlarged by new sections on Q-switching and resonators with internal phase/amplitude control. In addition, the whole book has been brought up-to-date.

  20. A resonant ionization laser ion source at ORNL

    Energy Technology Data Exchange (ETDEWEB)

    Liu, Y.; Stracener, D.W.

    2016-06-01

    Multi-step resonance laser ionization has become an essential tool for the production of isobarically pure radioactive ion beams at the isotope separator on-line (ISOL) facilities around the world. A resonant ionization laser ion source (RILIS) has been developed for the former Holifield Radioactive Ion Beam Facility (HRIBF) of Oak Ridge National Laboratory. The RILIS employs a hot-cavity ion source and a laser system featuring three grating-tuned and individually pumped Ti:Sapphire lasers, especially designed for stable and simple operation. The RILIS has been installed at the second ISOL production platform of former HRIBF and has successfully provided beams of exotic neutron-rich Ga isotopes for beta decay studies. This paper reports the features, advantages, limitations, and on-line and off-line performance of the RILIS.

  1. Current developments with TRIUMF’s titanium-sapphire laser based resonance ionization laser ion source

    Energy Technology Data Exchange (ETDEWEB)

    Lassen, J., E-mail: LASSEN@triumf.ca; Li, R. [TRIUMF (Canada); Raeder, S. [GSI Helmholtzzentrum für Schwerionenforschung GmbH (Germany); Zhao, X.; Dekker, T. [TRIUMF (Canada); Heggen, H. [GSI Helmholtzzentrum für Schwerionenforschung GmbH (Germany); Kunz, P.; Levy, C. D. P.; Mostanmand, M.; Teigelhöfer, A.; Ames, F. [TRIUMF (Canada)

    2017-11-15

    Developments at TRIUMF’s isotope separator and accelerator (ISAC) resonance ionization laser ion source (RILIS) in the past years have concentrated on increased reliability for on-line beam delivery of radioactive isotopes to experiments, as well as increasing the number of elements available through resonance ionization and searching for ionization schemes with improved efficiency. The current status of these developments is given with a list of two step laser ionization schemes implemented recently.

  2. Self-optimizing approach for automated laser resonator alignment

    Science.gov (United States)

    Brecher, C.; Schmitt, R.; Loosen, P.; Guerrero, V.; Pyschny, N.; Pavim, A.; Gatej, A.

    2012-02-01

    Nowadays, the assembly of laser systems is dominated by manual operations, involving elaborate alignment by means of adjustable mountings. From a competition perspective, the most challenging problem in laser source manufacturing is price pressure, a result of cost competition exerted mainly from Asia. From an economical point of view, an automated assembly of laser systems defines a better approach to produce more reliable units at lower cost. However, the step from today's manual solutions towards an automated assembly requires parallel developments regarding product design, automation equipment and assembly processes. This paper introduces briefly the idea of self-optimizing technical systems as a new approach towards highly flexible automation. Technically, the work focuses on the precision assembly of laser resonators, which is one of the final and most crucial assembly steps in terms of beam quality and laser power. The paper presents a new design approach for miniaturized laser systems and new automation concepts for a robot-based precision assembly, as well as passive and active alignment methods, which are based on a self-optimizing approach. Very promising results have already been achieved, considerably reducing the duration and complexity of the laser resonator assembly. These results as well as future development perspectives are discussed.

  3. Highly sensitive and selective determination of fluorine ion by graphene oxide/nanogold resonance Rayleigh scattering-energy transfer analytical platform.

    Science.gov (United States)

    Liang, Aihui; Peng, Jing; Liu, Qingye; Wen, Guiqing; Lu, Zhujun; Jiang, Zhiliang

    2015-08-15

    In pH 4.0 acetate buffer solution, fluorine ions react with fluorine reagent (FR) and La(III) to generate blue ternary complex that exhibited strong absorption at about 370 nm. Upon addition of graphene oxide/nanogold (GO/NG) as resonance Rayleigh scattering (RRS) spectral probe with strong RRS peak at 370 nm, the color changed to gray, and the RRS intensity decreased with the increase of fluorine ion concentration due to the RRS energy transfer (RRSET) from GO/NG to the complex. Under the selected condition, the decreased RRS peak ΔI370 nm was linear to fluorine ion concentration in the range of 6.0 × 10(-8)-1.3 × 10(-5)mol/L, with a detection limit of 3.0 × 10(-8)mol/L F(-). This RRSET method was applied to the analysis of fluorine in toothpaste and water samples, with satisfactory results. Copyright © 2015 Elsevier Ltd. All rights reserved.

  4. Time-Resolved Analysis of a Highly Sensitive Förster Resonance Energy Transfer Immunoassay Using Terbium Complexes as Donors and Quantum Dots as Acceptors

    Directory of Open Access Journals (Sweden)

    Niko Hildebrandt

    2007-01-01

    Full Text Available CdSe/ZnS core/shell quantum dots (QDs are used as efficient Förster Resonance Energy Transfer (FRET acceptors in a time-resolved immunoassays with Tb complexes as donors providing a long-lived luminescence decay. A detailed decay time analysis of the FRET process is presented. QD FRET sensitization is evidenced by a more than 1000-fold increase of the QD luminescence decay time reaching ca. 0.5 milliseconds, the same value to which the Tb donor decay time is quenched due to FRET to the QD acceptors. The FRET system has an extremely large Förster radius of approx. 100 Å and more than 70% FRET efficiency with a mean donor-acceptor distance of ca. 84 Å, confirming the applied biotin-streptavidin binding system. Time-resolved measurement allows for suppression of short-lived emission due to background fluorescence and directly excited QDs. By this means a detection limit of 18 attomol QDs within the immunoassay is accomplished, an improvement of more than two orders of magnitude compared to commercial systems.

  5. Design of high power solid-state pulsed laser resonators

    International Nuclear Information System (INIS)

    Narro, R.; Ponce, L.; Arronte, M.

    2009-01-01

    Methods and configurations for the design of high power solid-state pulsed laser resonators, operating in free running, are presented. For fundamental mode high power resonators, a method is proposed for the design of a resonator with joined stability zones. In the case of multimode resonators, two configurations are introduced for maximizing the laser overall efficiency due to the compensation of the astigmatism induced by the excitation. The first configuration consists in a triangular ring resonator. The results for this configuration are discussed theoretically, showing that it is possible to compensate the astigmatism of the thermal lens virtually in a 100%; however this is only possible for a specific pumping power. The second configuration proposes a dual-active medium resonator, rotated 90 degree one from the other around the optical axis, where each active medium acts as an astigmatic lens of the same dioptric power. The reliability of this configuration is corroborated experimentally using a Nd:YAG dual-active medium resonator. It is found that in the pumping power range where the astigmatism compensation is possible, the overall efficiency is constant, even when increasing the excitation power with the consequent increase of the thermal lens dioptric power. (Author)

  6. Thin disk laser with unstable resonator and reduced output coupler

    Science.gov (United States)

    Gavili, Anwar; Shayganmanesh, Mahdi

    2018-05-01

    In this paper, feasibility of using unstable resonator with reduced output coupling in a thin disk laser is studied theoretically. Unstable resonator is modeled by wave-optics using Collins integral and iterative method. An Yb:YAG crystal with 250 micron thickness is considered as a quasi-three level active medium and modeled by solving rate equations of energy levels populations. The amplification of laser beam in the active medium is calculated based on the Beer-Lambert law and Rigrod method. Using generalized beam parameters method, laser beam parameters like, width, divergence, M2 factor, output power as well as near and far-field beam profiles are calculated for unstable resonator. It is demonstrated that for thin disk laser (with single disk) in spite of the low thickness of the disk which leads to low gain factor, it is possible to use unstable resonator (with reduced output coupling) and achieve good output power with appropriate beam quality. Also, the behavior of output power and beam quality versus equivalent Fresnel number is investigated and optimized value of output coupling for maximum output power is achieved.

  7. Babinet principle and diffraction losses in laser resonators

    International Nuclear Information System (INIS)

    Kubarev, V V

    2000-01-01

    A simple analytical technique, based on the Babinet principle, for calculating low diffraction losses of different kinds in stable resonators is described. The technique was verified by comparison with the known numerical and analytical calculations of the losses in specific diffraction problems. (laser applications and other topics in quantum electronics)

  8. Resonant excitation of uranium atoms by an argon ion laser

    Energy Technology Data Exchange (ETDEWEB)

    Maeyama, H; Morikawa, M; Aihara, Y; Mochizuki, T; Yamanaka, C [Osaka Univ. (Japan)

    1979-03-01

    Photoionization of uranium atoms by UV lines, 3511 A and 3345 A, of an argon ion laser was observed and attributed due to resonant two-photon ionization. The dependence of the photoion currents on laser power was measured in focusing and non-focusing modes of laser beam, which has enabled us to obtain an absorption cross section and an ionization cross section independently. The orders of magnitude of these cross sections averaged over the fine structure were determined to be 10/sup -14/ cm/sup 2/ and 10/sup -17/ cm/sup 2/ respectively from a rate equation model. Resonance between 3511-A laser line and the absorption line of uranium isotopes was also confirmed by the ionization spectra obtained by near-single-frequency operation of the ion laser, which allowed the isotopic selective excitation of the uranium atoms. The maximum value of the enrichment of /sup 235/U was about 14%. The isotope separation of uranium atoms by this resonant excitation has been discussed.

  9. A highly sensitive fluorescence resonance energy transfer aptasensor for staphylococcal enterotoxin B detection based on exonuclease-catalyzed target recycling strategy

    International Nuclear Information System (INIS)

    Wu, Shijia; Duan, Nuo; Ma, Xiaoyuan; Xia, Yu; Wang, Hongxin; Wang, Zhouping

    2013-01-01

    Graphical abstract: -- Highlights: •An ultrasensitive FRET aptasensor was developed for staphylococcal enterotoxin B determination. •SEB was recognized by SEB aptamer with high affinity and specificity. •The Mn 2+ doped NaYF 4 :Yb/Er UCNPs used as donor to quencher dye (BHQ 3 ) in new FRET. •The fluorescence intensity was prominently amplified using an exonuclease-catalyzed target recycling strategy. -- Abstract: An ultrasensitive fluorescence resonance energy transfer (FRET) bioassay was developed to detect staphylococcal enterotoxin B (SEB), a low molecular exotoxin, using an aptamer-affinity method coupled with upconversion nanoparticles (UCNPs)-sensing, and the fluorescence intensity was prominently enhanced using an exonuclease-catalyzed target recycling strategy. To construct this aptasensor, both fluorescence donor probes (complementary DNA 1 –UCNPs) and fluorescence quencher probes (complementary DNA 2 –Black Hole Quencher 3 (BHQ 3 )) were hybridized to an SEB aptamer, and double-strand oligonucleotides were fabricated, which quenched the fluorescence of the UCNPs via FRET. The formation of an aptamer–SEB complex in the presence of the SEB analyte resulted in not only the dissociation of aptamer from the double-strand DNA but also both the disruption of the FRET system and the restoration of the UCNPs fluorescence. In addition, the SEB was liberated from the aptamer–SEB complex using exonuclease I, an exonuclease specific to single-stranded DNA, for analyte recycling by selectively digesting a particular DNA (SEB aptamer). Based on this exonuclease-catalyzed target recycling strategy, an amplified fluorescence intensity could be produced using different SEB concentrations. Using optimized experimental conditions produced an ultrasensitive aptasensor for the detection of SEB, with a wide linear range of 0.001–1 ng mL −1 and a lower detection limit (LOD) of 0.3 pg mL −1 SEB (at 3σ). The fabricated aptasensor was used to measure SEB in a

  10. Modeling laser brightness from cross Porro prism resonators

    Science.gov (United States)

    Forbes, Andrew; Burger, Liesl; Litvin, Igor Anatolievich

    2006-08-01

    Laser brightness is a parameter often used to compare high power laser beam delivery from various sources, and incorporates both the power contained in the particular mode, as well as the propagation of that mode through the beam quality factor, M2. In this study a cross Porro prism resonator is considered; crossed Porro prism resonators have been known for some time, but until recently have not been modeled as a complete physical optics system that allows the modal output to be determined as a function of the rotation angle of the prisms. In this paper we consider the diffraction losses as a function of the prism rotation angle relative to one another, and combine this with the propagation of the specific modes to determine the laser output brightness as a function of the prism orientation.

  11. Fundamentals of metasurface lasers based on resonant dark states

    International Nuclear Information System (INIS)

    Droulias, Sotiris; Technology - Hellas; Jain, Aditya; Koschny, Thomas; Soukoulis, Costas M.; Technology - Hellas; Ames Laboratory and Iowa State University, Ames, IA

    2017-01-01

    Recently, our group proposed a metamaterial laser design based on explicitly coupled dark resonant states in low-loss dielectrics, which conceptually separates the gain-coupled resonant photonic state responsible for macroscopic stimulated emission from the coupling to specific free-space propagating modes, allowing independent adjustment of the lasing state and its coherent radiation output. Due to this functionality, it is now possible to make lasers that can overcome the trade-off between system dimensions and Q factor, especially for surface emitting lasers with deeply subwavelength thickness. In this paper, we give a detailed discussion of the key functionality and benefits of this design, such as radiation damping tunability, directionality, subwavelength integration, and simple layer-by-layer fabrication. Finally, we examine in detail the fundamental design tradeoffs that establish the principle of operation and must be taken into account and give guidance for realistic implementations.

  12. Gas breakdown at cyclotron resonance with a submillimeter laser

    International Nuclear Information System (INIS)

    Hacker, M.P.; Temkin, R.J.; Lax, B.

    1976-01-01

    A pulsed 496-μm CH 3 F laser is used to produce gas breakdown in He at pressures between 1 and 300 Torr in an intense longitudinal magnetic field. Breakdown is detected by the observation of visible light when the electron cyclotron frequency (eB/m) equals the laser frequency, which occurs at B=216 kG for lambda=496 μm. At the lowest helium pressures and near cyclotron resonance, the focused laser intensity of 40 kW/cm 2 gives rise to very large electron heating rates, well beyond the limit of validity of conventional equilibrium breakdown theory. The observed result is an intensity-dependent resonant linewidth, much larger than predicted by equilibrium theories

  13. UV Resonant Raman Spectrometer with Multi-Line Laser Excitation

    Science.gov (United States)

    Lambert, James L.; Kohel, James M.; Kirby, James P.; Morookian, John Michael; Pelletier, Michael J.

    2013-01-01

    A Raman spectrometer employs two or more UV (ultraviolet) laser wavel engths to generate UV resonant Raman (UVRR) spectra in organic sampl es. Resonant Raman scattering results when the laser excitation is n ear an electronic transition of a molecule, and the enhancement of R aman signals can be several orders of magnitude. In addition, the Ra man cross-section is inversely proportional to the fourth power of t he wavelength, so the UV Raman emission is increased by another fact or of 16, or greater, over visible Raman emissions. The Raman-scatter ed light is collected using a high-resolution broadband spectrograph . Further suppression of the Rayleigh-scattered laser light is provi ded by custom UV notch filters.

  14. Differential interferometer for measurement of displacement of laser resonator mirrors

    Science.gov (United States)

    Macúchová, Karolina; Němcová, Šárka; Hošek, Jan

    2015-01-01

    This paper covers a description and a technique of a possible optical method of mode locking within a laser resonator. The measurement system is a part of instrumentation of laser-based experiment OSQAR at CERN. The OSQAR experiment aims at search of axions, axion-like particles and measuring of ultra-fine vacuum magnetic birefringence. It uses a laser resonator to enhance the coupling constant of hypothetical photon-to-axion conversion. The developed locking-in technique is based on differential interferometry. Signal obtained from the measurement provide crucial information for adaptive control of the locking-in of the resonator in real time. In this paper we propose several optical setups used for measurement and analysis of mutual position of the resonator mirrors. We have set up a differential interferometer under our laboratory conditions. We have done measurements with hemi-spherical cavity resonator detuned with piezo crystals. The measurement was set up in a single plane. Laser light was directed through half-wave retarder to a polarizing beam splitter and then converted to circular polarization by lambda/4 plates. After reflection at the mirrors, the beam is recombined in a beam splitter, sent to analyser and non-polarizing beam splitter and then inspected by two detectors with mutually perpendicular polarizers. The 90 degrees phase shift between the two arms allows precise analysis of a mutual distance change of the mirrors. Because our setup was sufficiently stable, we were able to measure the piezo constant and piezo hysteresis. The final goal is to adapt the first prototype to 23 m resonator and measure the displacement in two planes.

  15. Unstable Resonator Mid-Infrared Laser Sources

    Science.gov (United States)

    2016-02-26

    effective refractive indices of the guided mode at the grating ridge and groove were calcu- lated using a 4-layer slab waveguide model with a top clad... waterfall plot of the spectra. This DFB laser device demonstrated a continuous, mode-hop-free, tuning range of 80 nm, from 3057 to 3137 nm at ~2.5...curve is a quadratic fit. The inset shows the grating normal pump configuration (GNC). (b) Waterfall plot of the individual spectra vs. pump position

  16. In-Source Laser Resonance Ionization at ISOL Facilities

    CERN Document Server

    Marsh, Bruce; Feddosseev, Valentin

    Resonance ionization laser ion source development has been carried out at two radioactive ion beam facilities: ISOLDE (CERN, Switzerland) and the IGISOL facility (Jyvaskyla, Finland). The scope of the Resonance Ionization Laser Ion Source has been extended to 27 elements with the development of new three-step ionization schemes for Sb, Sc, Dy, Y and Au. The efficiencies were determined to be in the range of 2 - 20 %. Additionally, a new two-step ionization scheme has been developed for bismuth in an off-line atomic beam unit. The scheme relies on ionization via a strong and broad auto-ionizing resonance at an energy of 63196.79 cm$^{−1}$. This scheme may offer an improvement over the existing RILIS efficiency and will be more convenient for use during resonance ionization spectroscopy of Bi isotopes. The RILIS can be used as a spectroscopic tool to probe features such as the hyperfine structures and the isotope-shifts of radioisotopes with low production rates. By coupling a laser scanning process that dire...

  17. Low-Cost Miniaturized Laser Heterodyne Radiometer for Highly Sensitive Detection of CO2 and CH4 in the Atmospheric Column

    Science.gov (United States)

    Wilson, Emily L.; McLinden, Matthew L.; Miller, J. Houston

    2011-01-01

    We present a new passive ground-network instrument capable of measuring carbon dioxide (CO2) at 1.57 microns and methane (CH4) at 1.62 microns -- key for validation of OCO-2, ASCENDS, OCO-3, and GOSAT. Designed to piggy-back on an AERONET sun tracker (AERONET is a global network of more than 450 aerosol sensing instruments), this instrument could be rapidly deployed into the established AERONET network of ground sensors. Because aerosols induce a radiative effect that influences terrestrial carbon exchange, this simultaneous measure of aerosols and carbon cycle gases offers a uniquely comprehensive approach. This instrument is a variation of a laser heterodyne radiometer (LHR) that leverages recent advances in telecommunications lasers to miniaturize the instrument (the current version fits in a carry-on suitcase). In this technique, sunlight that has undergone absorption by the trace gas is mixed with laser light at a frequency matched to a trace gas absorption feature in the infrared (IR). Mixing results in a beat signal in the RF (radio frequency) region that can be related to the atmospheric concentration. By dividing this RF signal into a filter bank, concentrations at different altitudes can be resolved. For a one second integration, we estimate column sensitivities of 0.1 ppmv for CO2, and <1 ppbv for CH4.

  18. Dynamical resonance shift and unification of resonances in short-pulse laser-cluster interaction

    Science.gov (United States)

    Mahalik, S. S.; Kundu, M.

    2018-06-01

    Pronounced maximum absorption of laser light irradiating a rare-gas or metal cluster is widely expected during the linear resonance (LR) when Mie-plasma wavelength λM of electrons equals the laser wavelength λ . On the contrary, by performing molecular dynamics (MD) simulations of an argon cluster irradiated by short 5-fs (FWHM) laser pulses it is revealed that, for a given laser pulse energy and a cluster, at each peak intensity there exists a λ —shifted from the expected λM—that corresponds to a unified dynamical LR at which evolution of the cluster happens through very efficient unification of possible resonances in various stages, including (i) the LR in the initial time of plasma creation, (ii) the LR in the Coulomb expanding phase in the later time, and (iii) anharmonic resonance in the marginally overdense regime for a relatively longer pulse duration, leading to maximum laser absorption accompanied by maximum removal of electrons from cluster and also maximum allowed average charge states for the argon cluster. Increasing the laser intensity, the absorption maxima is found to shift to a higher wavelength in the band of λ ≈(1 -1.5 ) λM than permanently staying at the expected λM. A naive rigid sphere model also corroborates the wavelength shift of the absorption peak as found in MD and unequivocally proves that maximum laser absorption in a cluster happens at a shifted λ in the marginally overdense regime of λ ≈(1 -1.5 ) λM instead of λM of LR. The present study is important for guiding an optimal condition laser-cluster interaction experiment in the short-pulse regime.

  19. An improved prism for use in laser resonators

    Science.gov (United States)

    Richards, J.

    1981-08-01

    The use of compound total internal reflection prisms rather than Porro prisms in polarisation coupled lasers is proposed. Performance advantages resulting from the use of these prisms include higher output without the need to bias the Pockels cell, ability to give a larger range of output coupling and independence of performance on the refractive index of the prism. In conventional Q-switched lasers the use of the prism at the Pockels cell end of the resonator instead of the usual 100% reflecting mirror also leads to some advantages including better hold-off, elimination of the need to bias the Pockels cell and insensitivity in one plane to angular misalignment.

  20. Laser Beam and Resonator Calculations on Desktop Computers.

    Science.gov (United States)

    Doumont, Jean-Luc

    There is a continuing interest in the design and calculation of laser resonators and optical beam propagation. In particular, recently, interest has increased in developing concepts such as one-sided unstable resonators, supergaussian reflectivity profiles, diode laser modes, beam quality concepts, mode competition, excess noise factors, and nonlinear Kerr lenses. To meet these calculation needs, I developed a general-purpose software package named PARAXIA ^{rm TM}, aimed at providing optical scientists and engineers with a set of powerful design and analysis tools that provide rapid and accurate results and are extremely easy to use. PARAXIA can handle separable paraxial optical systems in cartesian or cylindrical coordinates, including complex-valued and misaligned ray matrices, with full diffraction effects between apertures. It includes the following programs:. ABCD provides complex-valued ray-matrix and gaussian -mode analyses for arbitrary paraxial resonators and optical systems, including astigmatism and misalignment in each element. This program required that I generalize the theory of gaussian beam propagation to the case of an off-axis gaussian beam propagating through a misaligned, complex -valued ray matrix. FRESNEL uses FFT and FHT methods to propagate an arbitrary wavefront through an arbitrary paraxial optical system using Huygens' integral in rectangular or radial coordinates. The wavefront can be multiplied by an arbitrary mirror profile and/or saturable gain sheet on each successive propagation through the system. I used FRESNEL to design a one-sided negative-branch unstable resonator for a free -electron laser, and to show how a variable internal aperture influences the mode competition and beam quality in a stable cavity. VSOURCE implements the virtual source analysis to calculate eigenvalues and eigenmodes for unstable resonators with both circular and rectangular hard-edged mirrors (including misaligned rectangular systems). I used VSOURCE to

  1. Tuning excitation laser wavelength for secondary resonance in low-intensity phase-selective laser-induced breakdown spectroscopy for in-situ analytical measurement of nanoaerosols

    Science.gov (United States)

    Xiong, Gang; Li, Shuiqing; Tse, Stephen D.

    2018-02-01

    In recent years, a novel low-intensity phase-selective laser-induced breakdown spectroscopy (PS-LIBS) technique has been developed for unique elemental-composition identification of aerosolized nanoparticles, where only the solid-phase nanoparticles break down, forming nanoplasmas, without any surrounding gas-phase breakdown. Additional work has demonstrated that PS-LIBS emissions can be greatly enhanced with secondary resonant excitation by matching the excitation laser wavelength with an atomic transition line in the formed nanoplasma, thereby achieving low limits of detection. In this work, a tunable dye laser is employed to investigate the effects of excitation wavelength and irradiance on in-situ PS-LIBS measurements of TiO2 nanoaerosols. The enhancement factor by resonant excitation can be 220 times greater than that for non-resonant cases under similar conditions. Moreover, the emitted spectra are unique for the selected resonant transition lines for a given element, suggesting the potential to make precise phase-selective and analyte-selective measurements of nanoparticles in a multicomponent multiphase system. The enhancement factor by resonant excitation is highly sensitive to excitation laser wavelength, with narrow excitation spectral windows, i.e., 0.012 to 0.023 nm (FWHM, full width at half maximum) for Ti (I) neutral atomic lines, and 0.051 to 0.139 nm (FWHM) for Ti (II) single-ionized atomic lines. Boltzmann analysis of the emission intensities, temporal response of emissions, and emission dependence on excitation irradiance are investigated to understand aspects of the generated nanoplasmas such as temperature, local thermodynamic equilibrium (LTE), and excitation mechanism.

  2. Single-mode Brillouin fiber laser passively stabilized at resonance frequency with self-injection locked pump laser

    International Nuclear Information System (INIS)

    Spirin, V V; Lopez-Mercado, C A; Megret, P; Fotiadi, A A

    2012-01-01

    We demonstrate a single-mode Brillouin fiber ring laser, which is passively stabilized at pump resonance frequency by using self-injection locking of semiconductor pump laser. Resonance condition for Stokes radiation is achieved by length fitting of Brillouin laser cavity. The laser generate single-frequency Stokes wave with linewidth less than 0.5 kHz using approximately 17-m length cavity

  3. Generation of low-energy muons with laser resonant ionization

    International Nuclear Information System (INIS)

    Matsuda, Y.; Bakule, P.; Iwasaki, M.; Matsuzaki, T.; Miyake, Y.; Ikedo, Y.; Strasser, P.; Shimomura, K.; Makimura, S.; Nagamine, K.

    2006-01-01

    We have constructed a low-energy muSR spectrometer at RIKEN-RAL muon facility in ISIS, the UK. With low-background of pulsed muon beam, and short pulse width from laser resonant ionization method, it is hoped this instrument will open new possibilities for studies of material sciences with muon beam. It is enphasized that this method is well suited to the facility where intense pulsed proton beam is available

  4. High-accuracy and high-sensitivity spectroscopic measurement of dinitrogen pentoxide (N2O5) in an atmospheric simulation chamber using a quantum cascade laser.

    Science.gov (United States)

    Yi, Hongming; Wu, Tao; Lauraguais, Amélie; Semenov, Vladimir; Coeur, Cecile; Cassez, Andy; Fertein, Eric; Gao, Xiaoming; Chen, Weidong

    2017-12-04

    A spectroscopic instrument based on a mid-infrared external cavity quantum cascade laser (EC-QCL) was developed for high-accuracy measurements of dinitrogen pentoxide (N 2 O 5 ) at the ppbv-level. A specific concentration retrieval algorithm was developed to remove, from the broadband absorption spectrum of N 2 O 5 , both etalon fringes resulting from the EC-QCL intrinsic structure and spectral interference lines of H 2 O vapour absorption, which led to a significant improvement in measurement accuracy and detection sensitivity (by a factor of 10), compared to using a traditional algorithm for gas concentration retrieval. The developed EC-QCL-based N 2 O 5 sensing platform was evaluated by real-time tracking N 2 O 5 concentration in its most important nocturnal tropospheric chemical reaction of NO 3 + NO 2 ↔ N 2 O 5 in an atmospheric simulation chamber. Based on an optical absorption path-length of L eff = 70 m, a minimum detection limit of 15 ppbv was achieved with a 25 s integration time and it was down to 3 ppbv in 400 s. The equilibrium rate constant K eq involved in the above chemical reaction was determined with direct concentration measurements using the developed EC-QCL sensing platform, which was in good agreement with the theoretical value deduced from a referenced empirical formula under well controlled experimental conditions. The present work demonstrates the potential and the unique advantage of the use of a modern external cavity quantum cascade laser for applications in direct quantitative measurement of broadband absorption of key molecular species involved in chemical kinetic and climate-change related tropospheric chemistry.

  5. Near resonant absorption by atoms in intense fluctuating laser fields

    International Nuclear Information System (INIS)

    Smith, S.J.

    1994-01-01

    The objective of this program was to make quantitative measurements of the effects of higher-order phase/frequency correlations in a laser beam on nonlinear optical absorption processes in atoms. The success of this program was due in large part to a unique experimental capability for modulating the extracavity beam of a stabilized (approx-lt 200 kHz) continuous-wave laser with statistically-well-characterized stochastic phase (or frequency) fluctuations, in order to synthesize laser bandwidths to ∼20 MHz (depending on noise amplitude), with profiles variable between Gaussian and Lorentzian (depending on noise bandwidth). Laser driven processes investigated included the following: (1) the optical Autler-Towns effect in the 3S 1/2 (F = 2, M F = 2) → 3P 3/2 (F = 3, M F = 3) two- level Na resonance, using a weak probe to the 4D 5/2 level; (2) the variance and spectra of fluorescence intensity fluctuations in the two-level Na resonance; (3) the Hanle effect in the 1 S 0 - 3 P 1 , transition at λ = 555.6 nm in 174 Yb; (4) absorption (and gain) of a weak probe, when the probe is a time-delayed replica of the resonant (with the two-level Na transition) pump laser; and (5) four-wave-mixing in a phase-conjugate geometry, in a sodium cell, and, finally, in a diffuse atomic sodium beam. The experimental results from these several studies have provided important confirmation of advanced theoretical methods

  6. Interference of laser-induced resonances in the continuous structures of a helium atom

    International Nuclear Information System (INIS)

    Magunov, A I; Strakhova, S I

    2003-01-01

    Coherent effects in the interference of overlapping laser-induced resonances in helium atoms are considered. The simultaneous action of single-mode radiation of the 294-nm second harmonic of a cw dye laser and a 1064-nm Nd:YAG laser on helium atoms provides the overlap of two resonances induced by transitions from the 1s2s 1 S and 1s4s 1 S helium levels. The shape of the overlapping laser-induced resonances in the rotating-wave approximation is described by analytic expressions, which depend on the laser radiation intensities and the ratio of laser frequencies. (nonlinear optical phenomena)

  7. Resonant laser printing of structural colors on high-index dielectric metasurfaces

    DEFF Research Database (Denmark)

    Zhu, Xiaolong; Yan, Wei; Levy, Uriel

    2017-01-01

    -dependent resonances. Strong on-resonance energy absorption under pulsed laser irradiation locally elevates the lattice temperature (exceeding 1200 K) in an ultrashort time scale (1 ns). This forms the basis for resonant laser printing, where rapid melting allows for surface energy-driven morphology changes...

  8. Practical and highly sensitive elemental analysis for aqueous samples containing metal impurities employing electrodeposition on indium-tin oxide film samples and laser-induced shock wave plasma in low-pressure helium gas.

    Science.gov (United States)

    Kurniawan, Koo Hendrik; Pardede, Marincan; Hedwig, Rinda; Abdulmadjid, Syahrun Nur; Lahna, Kurnia; Idris, Nasrullah; Jobiliong, Eric; Suyanto, Hery; Suliyanti, Maria Margaretha; Tjia, May On; Lie, Tjung Jie; Lie, Zener Sukra; Kurniawan, Davy Putra; Kagawa, Kiichiro

    2015-09-01

    We have conducted an experimental study exploring the possible application of laser-induced breakdown spectroscopy (LIBS) for practical and highly sensitive detection of metal impurities in water. The spectrochemical measurements were carried out by means of a 355 nm Nd-YAG laser within N2 and He gas at atmospheric pressures as high as 2 kPa. The aqueous samples were prepared as thin films deposited on indium-tin oxide (ITO) glass by an electrolysis process. The resulting emission spectra suggest that concentrations at parts per billion levels may be achieved for a variety of metal impurities, and it is hence potentially feasible for rapid inspection of water quality in the semiconductor and pharmaceutical industries, as well as for cooling water inspection for possible leakage of radioactivity in nuclear power plants. In view of its relative simplicity, this LIBS equipment offers a practical and less costly alternative to the standard use of inductively coupled plasma-mass spectrometry (ICP-MS) for water samples, and its further potential for in situ and mobile applications.

  9. Resonant heating of a cluster plasma by intense laser light

    International Nuclear Information System (INIS)

    Antonsen, Thomas M. Jr.; Taguchi, Toshihiro; Gupta, Ayush; Palastro, John; Milchberg, Howard M.

    2005-01-01

    Gases of atomic clusters are interaction media for laser pulse propagation with properties useful for applications such as extreme ultraviolet (EUV) and x-ray microscopy, harmonic generation, EUV lithography, and laser plasma acceleration. To understand cluster heating and expansion, a series of two- and three-dimensional electrostatic particle in cell simulations of the explosion of argon clusters of diameter in the range 20 nm-53 nm have been preformed. The studies show that heating is dominated by a nonlinear, resonant absorption process that gives rise to a size-dependent intensity threshold for strong absorption and that controls the dielectric properties of the cluster. Electrons are first accelerated out from the cluster and then driven back into it by the combined effects of the laser field and the electrostatic field produced by the laser-driven charge separation. Above the intensity threshold for strong heating there is a dramatic increase in the production of energetic particles and harmonic radiation. The dielectric properties of a gas of clusters are determined by the ensemble average cluster polarizability. Individual electrons contribute to the polarizability differently depending on whether they are in the core of the cluster or in the outer edge. Consequently, there can be large fluctuations in polarizability during the heating of a cluster

  10. Stability of a short Rayleigh length laser resonator

    Directory of Open Access Journals (Sweden)

    P. P. Crooker

    2005-04-01

    Full Text Available Motivated by the prospect of constructing a short Rayleigh length free-electron laser in a high-vibration environment, we demonstrate the use of a collection of rays to study the effect of mirror vibration and distortion on the behavior of the fundamental optical mode of a cold-cavity resonator. We find that the ray collection accurately describes both on-axis and off-axis optical beams. We show that a tilt or transverse shift of a mirror causes the optical mode to rock about the original resonator axis, while a longitudinal mirror shift or a change in the mirror’s radius of curvature causes the beam diameter at a mirror to successively dilate and contract on the mirror. Results are in excellent agreement with analytic calculations and wave front propagation simulations as long as the mirrors remain large with respect to the beam diameter.

  11. A dye laser with a partial-selective resonator

    Energy Technology Data Exchange (ETDEWEB)

    Makogon, M M; Sukhanov, V B

    1977-04-01

    The possibility of controlling the width and spectral position of the generation line of an organic dye laser (Rhodamine 6Zh) whose resonator represents a combination of selective and non-selective channels is demonstrated. The selective channel entails an unsymmetrically mounted prism with whose angular displacement the spectral width can be changed within broad ranges; the non-selective channel maintains the resonator's quality at a sufficiently high level. An expression is given which makes it possible to determine the generation's spectral width when fixing the prism's angular position. The change in the rearrangement band was studied in relation to the qualities of the selective and non-selective channels as determined by the form of the active medium's amplification contour (a narrowing of the spectrum from 0.15 to 0.0019 nm led to a reduction of the rearrangement area from 38.4 to 28.3 nm).

  12. High-Sensitivity Temperature-Independent Silicon Photonic Microfluidic Biosensors

    Science.gov (United States)

    Kim, Kangbaek

    Optical biosensors that can precisely quantify the presence of specific molecular species in real time without the need for labeling have seen increased use in the drug discovery industry and molecular biology in general. Of the many possible optical biosensors, the TM mode Si biosensor is shown to be very attractive in the sensing application because of large field amplitude on the surface and cost effective CMOS VLSI fabrication. Noise is the most fundamental factor that limits the performance of sensors in development of high-sensitivity biosensors, and noise reduction techniques require precise studies and analysis. One such example stems from thermal fluctuations. Generally SOI biosensors are vulnerable to ambient temperature fluctuations because of large thermo-optic coefficient of silicon (˜2x10 -4 RIU/K), typically requiring another reference ring and readout sequence to compensate temperature induced noise. To address this problem, we designed sensors with a novel TM-mode shallow-ridge waveguide that provides both large surface amplitude for bulk and surface sensing. With proper design, this also provides large optical confinement in the aqueous cladding that renders the device athermal using the negative thermo-optic coefficient of water (~ --1x10-4RIU/K), demonstrating cancellation of thermo-optic effects for aqueous solution operation near 300K. Additional limitations resulting from mechanical actuator fluctuations, stability of tunable lasers, and large 1/f noise of lasers and sensor electronics can limit biosensor performance. Here we also present a simple harmonic feedback readout technique that obviates the need for spectrometers and tunable lasers. This feedback technique reduces the impact of 1/f noise to enable high-sensitivity, and a DSP lock-in with 256 kHz sampling rate can provide down to micros time scale monitoring for fast transitions in biomolecular concentration with potential for small volume and low cost. In this dissertation, a novel

  13. A homogeneous assay for highly sensitive detection of CaMV35S promoter in transgenic soybean by förster resonance energy transfer between nitrogen-doped graphene quantum dots and Ag nanoparticles

    Energy Technology Data Exchange (ETDEWEB)

    Li, Yaqi; Sun, Li [School of Food and Biological Engineering, Jiangsu University, Zhenjiang, 212013 (China); Qian, Jing [School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212013 (China); Wang, Chengke [School of Food and Biological Engineering, Jiangsu University, Zhenjiang, 212013 (China); Liu, Qian [School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212013 (China); Han, En [School of Food and Biological Engineering, Jiangsu University, Zhenjiang, 212013 (China); Hao, Nan [School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212013 (China); Zhang, Liuping [Sinograin Zhenjiang Grains & Oils Quality Testing Center Co., Ltd., Zhenjiang, 212013 (China); Cai, Jianrong, E-mail: jrcai@ujs.edu.cn [School of Food and Biological Engineering, Jiangsu University, Zhenjiang, 212013 (China); Wang, Kun, E-mail: wangkun@ujs.edu.cn [School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212013 (China)

    2016-12-15

    In this work, a novel homogeneous assay for DNA quantitative analysis based on förster resonance energy transfer (FRET) was developed for cauliflwer mosaic virus 35s (CaMV35S) promoter of transgenic soybean detection. The homogenous FRET of fluorescence signal was fabricated by DNA hybridization with probe modified nitrogen-doped graphene quantum dots (NGQDs) and silver nanoparticles (AgNPs), which acted the donor-acceptor pairs for the first time. The highly efficient FRET and unique properties of the NGQDs made the proposed FRET system as a functionalized detection platform for labelling of DNA. Upon the recognition of specific target DNA (tDNA), the FRET between NGQDs and AgNPs was triggered to produce fluorescence quenching, which could be used for tDNA detection. The fabricated homogeneous FRET assay displayed a wide linear range of 0.1–500.0 nM and a low limit of detection 0.03 nM for the detection of CaMV35S (S/N = 3). This proposed biosensor revealed high specificity to detect tDNA, with acceptable intra-assay precision and excellent stability. This method was successfully applied to identify the real sample of 0.5% containing transgenic soybean, which achieved the most of national law regulations. This assay was further validated by polymerase chain reaction as the genetically modified organisms, suggesting that the proposed FRET system is a feasible tool for the further daily genetically modified organism detection. - Highlights: • Both NGQDs and AgNPs were selected as the novel FRET donor-acceptor pairs. • The proposed homogeneous FRET assay was developed for CaMV35S detection. • The resulting method could identify 0.5% containing transgenic soybean sample. • This assay was inexpensive, simple and highly sensitive.

  14. Highly-sensitive aptasensor based on fluorescence resonance energy transfer between l-cysteine capped ZnS quantum dots and graphene oxide sheets for the determination of edifenphos fungicide.

    Science.gov (United States)

    Arvand, Majid; Mirroshandel, Aazam A

    2017-10-15

    With the advantages of excellent optical properties and biocompatibility, single-strand DNA-functionalized quantum dots have been widely applied in biosensing and bioimaging. A new aptasensor with easy operation, high sensitivity, and high selectivity was developed by immobilizing the aptamer on water soluble l-cysteine capped ZnS quantum dots (QDs). Graphene oxide (GO) sheets are mixed with the aptamer-QDs. Consequently, the aptamer-conjugated QDs bind to the GO sheets to form a GO/aptamer-QDs ensemble. This aptasensor enables the energy transfer based on a fluorescence resonance energy transfer (FRET) from the QDs to the GO sheets, quenching the fluorescence of QDs. The GO/aptamer-QDs ensemble assay acts as a "turn-on'' fluorescent sensor for edifenphos (EDI) detection. When GO was replaced by EDI, the fluorescence of QDs was restored and its intensity was proportional to the EDI concentration. This GO-based aptasensor under the optimum conditions exhibited excellent analytical performance for EDI determination, ranging from 5×10 -4 to 6×10 -3 mg L -1 with the detection limit of 1.3×10 -4 mgL -1 . Furthermore, the designed aptasensor exhibited excellent selectivity toward EDI compared to other pesticides and herbicides with similar structures such as diazinon, heptachlor, endrin, dieldrin, butachlor and chlordane. Good reproducibility and precision (RSD =3.9%, n =10) of the assay indicates the high potential of the aptasensor for quantitative trace analysis of EDI. Moreover, the results demonstrate the applicability of the aptasensor for monitoring EDI fungicide in spiked real samples. Copyright © 2017 Elsevier B.V. All rights reserved.

  15. A homogeneous assay for highly sensitive detection of CaMV35S promoter in transgenic soybean by förster resonance energy transfer between nitrogen-doped graphene quantum dots and Ag nanoparticles

    International Nuclear Information System (INIS)

    Li, Yaqi; Sun, Li; Qian, Jing; Wang, Chengke; Liu, Qian; Han, En; Hao, Nan; Zhang, Liuping; Cai, Jianrong; Wang, Kun

    2016-01-01

    In this work, a novel homogeneous assay for DNA quantitative analysis based on förster resonance energy transfer (FRET) was developed for cauliflwer mosaic virus 35s (CaMV35S) promoter of transgenic soybean detection. The homogenous FRET of fluorescence signal was fabricated by DNA hybridization with probe modified nitrogen-doped graphene quantum dots (NGQDs) and silver nanoparticles (AgNPs), which acted the donor-acceptor pairs for the first time. The highly efficient FRET and unique properties of the NGQDs made the proposed FRET system as a functionalized detection platform for labelling of DNA. Upon the recognition of specific target DNA (tDNA), the FRET between NGQDs and AgNPs was triggered to produce fluorescence quenching, which could be used for tDNA detection. The fabricated homogeneous FRET assay displayed a wide linear range of 0.1–500.0 nM and a low limit of detection 0.03 nM for the detection of CaMV35S (S/N = 3). This proposed biosensor revealed high specificity to detect tDNA, with acceptable intra-assay precision and excellent stability. This method was successfully applied to identify the real sample of 0.5% containing transgenic soybean, which achieved the most of national law regulations. This assay was further validated by polymerase chain reaction as the genetically modified organisms, suggesting that the proposed FRET system is a feasible tool for the further daily genetically modified organism detection. - Highlights: • Both NGQDs and AgNPs were selected as the novel FRET donor-acceptor pairs. • The proposed homogeneous FRET assay was developed for CaMV35S detection. • The resulting method could identify 0.5% containing transgenic soybean sample. • This assay was inexpensive, simple and highly sensitive.

  16. Opto-mechanical design of vacuum laser resonator for the OSQAR experiment

    Science.gov (United States)

    Hošek, Jan; Macúchová, Karolina; Nemcová, Šárka; Kunc, Štěpán.; Šulc, Miroslav

    2015-01-01

    This paper gives short overview of laser-based experiment OSQAR at CERN which is focused on search of axions and axion-like particles. The OSQAR experiment uses two experimental methods for axion search - measurement of the ultra-fine vacuum magnetic birefringence and a method based on the "Light shining through the wall" experiment. Because both experimental methods have reached its attainable limits of sensitivity we have focused on designing a vacuum laser resonator. The resonator will increase the number of convertible photons and their endurance time within the magnetic field. This paper presents an opto-mechanical design of a two component transportable vacuum laser resonator. Developed optical resonator mechanical design allows to be used as a 0.8 meter long prototype laser resonator for laboratory testing and after transportation and replacement of the mirrors it can be mounted on the LHC magnet in CERN to form a 20 meter long vacuum laser resonator.

  17. Laser-induced breakdown spectroscopy with laser irradiation resonant with vibrational transitions

    International Nuclear Information System (INIS)

    Khachatrian, Ani; Dagdigian, Paul J.

    2010-01-01

    An investigation of laser-induced breakdown spectroscopy (LIBS) of polymers, both in bulk form and spin coated on Si wafers, with laser irradiation in the mid-infrared spectral region is presented. Of particular interest is whether the LIBS signals are enhanced when the laser wavelength is resonant with a fundamental vibrational transition of the polymer. Significant increases in the LIBS signals were observed for irradiation on hydride stretch fundamental transitions, and the magnitude of the enhancement showed a strong dependence on the mode excited. The role of the substrate was investigated by comparison of results for bulk and spin-coated samples. The polymers investigated were Nylon 12 and poly(vinyl alcohol-co-ethylene).

  18. Isotopically selective RIMS of rare radionuclides by double-resonance excitation with cw lasers

    International Nuclear Information System (INIS)

    Bushaw, B.A.; Munley, J.T.

    1990-09-01

    Double-resonance, Resonance Ionization Mass Spectroscopy (RIMS) using two single-frequency dye lasers and a CO 2 laser for photoionization has been shown to be both extremely sensitive and highly selective. Measurements on the radioisotope 210 Pb have demonstrated optical selectivity in excess of 10 9 and detection limits of less than 1 femtogram

  19. Resonant laser techniques for combustion and flow diagnostics

    Energy Technology Data Exchange (ETDEWEB)

    Fritzon, Rolf

    1998-05-01

    This thesis presents results from two areas of research. Firstly, the resonant coherent laser techniques polarization spectroscopy (PS), degenerate four-wave mixing (DFWM) and stimulated emission (SE) have been developed in the general field of combustion diagnostics. Secondly, laser induced fluorescence (LIF) has been developed and applied for the visualization of mixture fractions in turbulent non reacting flows. PS was developed for instantaneous two-dimensional imaging of minor species in flames, the technique being demonstrated on OH and NO. Various aspects of imaging and of detection in general were investigated. Two-photon induced PS was demonstrated for the detection of NH{sub 3}, CO and N{sub 2} molecules. LIF was monitored simultaneously to allow a quantitative comparison between the techniques. Furthermore, PS and DFWM were developed for instantaneous two-dimensional OH temperature imaging. Through a novel experimental approach based on the use of a dual-wavelength dye laser and a diffraction grating the temperature imaging measurements were performed using only one laser and one CCD camera. A comparison between the two techniques was made. SE was through a crossed-beam arrangement developed for spatially resolved detection of flame species. Two-dimensional LIF was developed and applied for measuring mixture fractions in the shear layer between two co-flowing turbulent gaseous jets. The technique was further applied in a study of the mixing of a turbulent water jet impinging orthogonally onto a flat surface. Average concentration fields in the center-plane of the jet was compared with results from large eddy simulations and with data from the literature 221 refs, 48 figs, 5 tabs

  20. Cavity-enhanced resonant photoacoustic spectroscopy with optical feedback cw diode lasers: A novel technique for ultratrace gas analysis and high-resolution spectroscopy.

    Science.gov (United States)

    Hippler, Michael; Mohr, Christian; Keen, Katherine A; McNaghten, Edward D

    2010-07-28

    Cavity-enhanced resonant photoacoustic spectroscopy with optical feedback cw diode lasers (OF-CERPAS) is introduced as a novel technique for ultratrace gas analysis and high-resolution spectroscopy. In the scheme, a single-mode cw diode laser (3 mW, 635 nm) is coupled into a high-finesse linear cavity and stabilized to the cavity by optical feedback. Inside the cavity, a build-up of laser power to at least 2.5 W occurs. Absorbing gas phase species inside the cavity are detected with high sensitivity by the photoacoustic effect using a microphone embedded in the cavity. To increase sensitivity further, coupling into the cavity is modulated at a frequency corresponding to a longitudinal resonance of an organ pipe acoustic resonator (f=1.35 kHz and Q approximately 10). The technique has been characterized by measuring very weak water overtone transitions near 635 nm. Normalized noise-equivalent absorption coefficients are determined as alpha approximately 4.4x10(-9) cm(-1) s(1/2) (1 s integration time) and 2.6x10(-11) cm(-1) s(1/2) W (1 s integration time and 1 W laser power). These sensitivities compare favorably with existing state-of-the-art techniques. As an advantage, OF-CERPAS is a "zero-background" method which increases selectivity and sensitivity, and its sensitivity scales with laser power.

  1. Technology of discharge and laser resonators for high power CO2 lasers. Koshutsuryoku CO2 laser ni tsukawareru hoden reiki laser kyoshinki gijutsu

    Energy Technology Data Exchange (ETDEWEB)

    Takenaka, Y.; Kuzumoto, M. (Mitsubishi Electric Corp., Tokyo (Japan))

    1994-03-20

    This paper describes discharge excitation technology and resonator technology as basic technologies for high power CO2 lasers. As a result of progress in high-frequency power element techniques, the discharge excitation technology now generally uses laser excitation using AC discharge of capacity coupling type. Its representative example is silent discharge (SD) excitation. This is a system to excite laser by applying high voltages with as high frequency as 100 kHz to 1 MHz across a pair of electrodes covered with a dielectric material. The system maintains stability in discharge even if power supply voltage amplitude is modulated, and easily provides pulse outputs. Discharge excitation for diffusion cooled type CO2 laser generates a discharge in a gap with a gap length of about 2 mm, and can perform gas cooling by means of thermal conduction of gas, whereas a compact resonator can be fabricated. A resonator for the diffusion cooled type CO2 laser eliminates gas circulation and cooling systems, hence the device can be made more compact. A report has been given that several of these compact resonators were combined, from which a laser output of 85W was obtained by using RF discharge of 2kW. 43 refs., 21 figs.

  2. Resonant infrared pulsed laser deposition of a polyimide precursor

    Energy Technology Data Exchange (ETDEWEB)

    Dygert, N L; Schriver, K E; Jr, R F Haglund [Department of Physics and Astronomy and W M Keck Foundation Free-Electron Laser Centre, Vanderbilt University, Nashville TN 37235 (United States)

    2007-04-15

    Poly(amic acid) (PAA), a precursor to polyimide, was successfully deposited on substrates without reaching curing temperature, by resonant infrared pulsed laser ablation. The PAA was prepared by dissolving pyromellitic dianhydride and 4, 4' oxidianiline in the polar solvent Nmethyl pyrrolidinone (NMP). The PAA was deposited in droplet-like morphologies when ablation occurred in air, and in string-like moieties in the case of ablation in vacuum. In the as-deposited condition, the PAA was easily removed by washing with NMP; however, once cured thermally for thirty minutes, the PAA hardened, indicating the expected thermosetting property. Plume shadowgraphy showed very clear contrasts in the ablation mechanism between ablation of the solvent alone and the ablation of the PAA, even at low concentrations. A Wavelength dependence in plume velocity was also observed.

  3. Double resonance modulation characteristics of optically injection-locked Fabry–Perot lasers

    International Nuclear Information System (INIS)

    Dorogush, E S; Afonenko, A A

    2015-01-01

    The distributed resonator model is used to show the presence of several resonance responses on the modulation characteristic of optically injection-locked Fabry–Perot lasers. The positions of the resonance peaks on the modulation characteristic are determined by the resonator length and frequency detuning of optical injection. It is shown that an appropriate choice of the resonator length and injection locking conditions allows one to obtain efficient modulation in two ranges near 40 – 60 GHz or to increase the direct modulation bandwidth up to 50 GHz. (control of laser radiation parameters)

  4. Double resonance modulation characteristics of optically injection-locked Fabry–Perot lasers

    Energy Technology Data Exchange (ETDEWEB)

    Dorogush, E S; Afonenko, A A [Belarusian State University, Minsk (Belarus)

    2015-12-31

    The distributed resonator model is used to show the presence of several resonance responses on the modulation characteristic of optically injection-locked Fabry–Perot lasers. The positions of the resonance peaks on the modulation characteristic are determined by the resonator length and frequency detuning of optical injection. It is shown that an appropriate choice of the resonator length and injection locking conditions allows one to obtain efficient modulation in two ranges near 40 – 60 GHz or to increase the direct modulation bandwidth up to 50 GHz. (control of laser radiation parameters)

  5. Laser resonance ionization spectroscopy on lutetium for the MEDICIS project

    Energy Technology Data Exchange (ETDEWEB)

    Gadelshin, V., E-mail: gadelshin@uni-mainz.de [University of Mainz, Institute of Physics (Germany); Cocolios, T. [KU Leuven, Institute for Nuclear and Radiation Physics (Belgium); Fedoseev, V. [CERN, EN Department (Switzerland); Heinke, R.; Kieck, T. [University of Mainz, Institute of Physics (Germany); Marsh, B. [CERN, EN Department (Switzerland); Naubereit, P. [University of Mainz, Institute of Physics (Germany); Rothe, S.; Stora, T. [CERN, EN Department (Switzerland); Studer, D. [University of Mainz, Institute of Physics (Germany); Duppen, P. Van [KU Leuven, Institute for Nuclear and Radiation Physics (Belgium); Wendt, K. [University of Mainz, Institute of Physics (Germany)

    2017-11-15

    The MEDICIS-PROMED Innovative Training Network under the Horizon 2020 EU program aims to establish a network of early stage researchers, involving scientific exchange and active cooperation between leading European research institutions, universities, hospitals, and industry. Primary scientific goal is the purpose of providing and testing novel radioisotopes for nuclear medical imaging and radionuclide therapy. Within a closely linked project at CERN, a dedicated electromagnetic mass separator system is presently under installation for production of innovative radiopharmaceutical isotopes at the new CERN-MEDICIS laboratory, directly adjacent to the existing CERN-ISOLDE radioactive ion beam facility. It is planned to implement a resonance ionization laser ion source (RILIS) to ensure high efficiency and unrivaled purity in the production of radioactive ions. To provide a highly efficient ionization process, identification and characterization of a specific multi-step laser ionization scheme for each individual element with isotopes of interest is required. The element lutetium is of primary relevance, and therefore was considered as first candidate. Three two-step excitation schemes for lutetium atoms are presented in this work, and spectroscopic results are compared with data of other authors.

  6. Laser resonance ionization spectroscopy on lutetium for the MEDICIS project

    Science.gov (United States)

    Gadelshin, V.; Cocolios, T.; Fedoseev, V.; Heinke, R.; Kieck, T.; Marsh, B.; Naubereit, P.; Rothe, S.; Stora, T.; Studer, D.; Van Duppen, P.; Wendt, K.

    2017-11-01

    The MEDICIS-PROMED Innovative Training Network under the Horizon 2020 EU program aims to establish a network of early stage researchers, involving scientific exchange and active cooperation between leading European research institutions, universities, hospitals, and industry. Primary scientific goal is the purpose of providing and testing novel radioisotopes for nuclear medical imaging and radionuclide therapy. Within a closely linked project at CERN, a dedicated electromagnetic mass separator system is presently under installation for production of innovative radiopharmaceutical isotopes at the new CERN-MEDICIS laboratory, directly adjacent to the existing CERN-ISOLDE radioactive ion beam facility. It is planned to implement a resonance ionization laser ion source (RILIS) to ensure high efficiency and unrivaled purity in the production of radioactive ions. To provide a highly efficient ionization process, identification and characterization of a specific multi-step laser ionization scheme for each individual element with isotopes of interest is required. The element lutetium is of primary relevance, and therefore was considered as first candidate. Three two-step excitation schemes for lutetium atoms are presented in this work, and spectroscopic results are compared with data of other authors.

  7. Significance of the Resonance Condition for Controlling the Seam Position in Laser-assisted TIG Welding

    Science.gov (United States)

    Emde, B.; Huse, M.; Hermsdorf, J.; Kaierle, S.; Wesling, V.; Overmeyer, L.; Kozakov, R.; Uhrlandt, D.

    As an energy-preserving variant of laser hybrid welding, laser-assisted arc welding uses laser powers of less than 1 kW. Recent studies have shown that the electrical conductivity of a TIG welding arc changes within the arc in case of a resonant interaction between laser radiation and argon atoms. This paper presents investigations on how to control the position of the arc root on the workpiece by means of the resonant interaction. Furthermore, the influence on the welding result is demonstrated. The welding tests were carried out on a cooled copper plate and steel samples with resonant and non-resonant laser radiation. Moreover, an analysis of the weld seam is presented.

  8. Assisted inhibition effect of acetylcholinesterase with n-octylphosphonic acid and application in high sensitive detection of organophosphorous pesticides by matrix-assisted laser desorption/ionization Fourier transform mass spectrometry.

    Science.gov (United States)

    Cai, Tingting; Zhang, Li; Wang, Haoyang; Zhang, Jing; Guo, Yinlong

    2011-11-14

    A simple and practical approach to improve the sensitivity of acetylcholinesterase (AChE)-inhibited method has been developed for monitoring organophosphorous (OP) pesticide residues. In this work, matrix-assisted laser desorption/ionization Fourier transform mass spectrometry (MALDI-FTMS) was used to detect AChE activity. Due to its good salt-tolerance and low sample consumption, MALDI-FTMS facilitates rapid and high-throughput screening of OP pesticides. Here we describe a new method to obtain low detection limits via employing external reagents. Among candidate compounds, n-octylphosphonic acid (n-Octyl-PA) displays assistant effect to enhance AChE inhibition by OP pesticides. In presence of n-Octyl-PA, the percentages of AChE inhibition still kept correlation with OP pesticide concentrations. The detection limits were improved significantly even by 10(2)-10(3) folds in comparison with conventional enzyme-inhibited methods. Different detection limits of OP pesticides with different toxicities were as low as 0.005 μg L(-1) for high toxic pesticides and 0.05 μg L(-1) for low toxic pesticides. Besides, the reliability of results from this method to analyze cowpea samples had been demonstrated by liquid-chromatography tandem mass spectrometry (LC-MS/MS). The application of this commercial available assistant agent shows great promise to detect OP compounds in complicated biological matrix and broadens the mind for high sensitivity detection of OP pesticide residues in agricultural products. Copyright © 2011 Elsevier B.V. All rights reserved.

  9. Application of laser resonance scattering to the study of high-temperature plasma-wall interaction

    International Nuclear Information System (INIS)

    Maeda, Mitsuo; Muraoka, Katsunori; Hamamoto, Makoto; Akazaki, Masanori; Miyazoe, Yasushi

    1981-01-01

    Studies on laser resonance scattering and its application to the study of high-temperature plasma-wall interaction are reviewed. The application of dye laser beam to resonant scattering method has been developed. This method is able to detect low density atoms. The fluorescent photon counts can be estimated for a two-level system and a three-level system. The S/N ratio, Which is in close connection with the detection limit, has been estimated. The doppler effect due to the thermal motion of atoms is taken into consideration. The calibration of the absolute number of atoms is necessary. Tunable coherent light is used as the light source for resonance scattering method. This is able to excite atoms strongly and to increase the detection efficiency. As dye lasers, a N 2 laser, a YAG laser, and a KrF excimer laser have been studied. In VUV region, rare gas or rare gas halide lasers can be used. The strong output power can be expected when the resonance lines of atoms meet the synchronizing region of the excimer laser. The resonance scattering method is applied to the detection of impurity metal atoms in plasma. The studies of laser systems for the detection of hydrogen atoms are also in progress. (Kato, T.)

  10. New possibilities for using laser polarimetry technology to study electron paramagnetic resonance

    Energy Technology Data Exchange (ETDEWEB)

    Aleksandrov, E V; Zapasskii, V S

    1982-01-01

    Optical methods of recording electron paramagnetic resonance which arose in the early 50's as applied to the problem of recording the magnetic resonance of excited atoms is at the present time widely used in studying the electron paramagnetic resonance of the ground and excited states of free atoms and paramagnetic centers in condensed media. At the present time attention is devoted to the additional possibilities of optical methods of electron paramagnetic resonance which are realized using laser sources.

  11. Optical Analysis of Grazing Incidence Ring Resonators for Free-Electron Lasers

    Science.gov (United States)

    Gabardi, David Richard

    1990-08-01

    The design of resonators for free-electron lasers (FELs) which are to operate in the soft x-ray/vacuum ultraviolet (XUV) region of the spectrum is complicated by the fact that, in this wavelength regime, normal incidence mirrors, which would otherwise be used for the construction of the resonators, generally have insufficient reflectivities for this purpose. However, the use of grazing incidence mirrors in XUV resonators offers the possibility of (1) providing sufficient reflectivity, (2) a lessening of the mirrors' thermal loads due to the projection of the laser beam onto an oblique surface, and (3) the preservation of the FEL's tunability. In this work, the behavior of resonators employing grazing incidence mirrors in ring type configurations is explored. In particular, two designs, each utilizing four off-axis conic mirrors and a number of flats, are examined. In order to specify the location, orientation, and surface parameters for the mirrors in these resonators, a design algorithm has been developed based upon the properties of Gaussian beam propagation. Two computer simulation methods are used to perform a vacuum stability analysis of the two resonator designs. The first method uses paraxial ray trace techniques with the resonators' thin lens analogues while the second uses the diffraction-based computer simulation code GLAD (General Laser Analysis and Design). The effects of mirror tilts and deviations in the mirror surface parameters are investigated for a number of resonators designed to propagate laser beams of various Rayleigh ranges. It will be shown that resonator stability decreases as the laser wavelength for which the resonator was designed is made smaller. In addition, resonator stability will also be seen to decrease as the amount of magnification the laser beam receives as it travels around the resonator is increased.

  12. An All-Solid-State High Repetiton Rate Titanium:Sapphire Laser System For Resonance Ionization Laser Ion Sources

    Science.gov (United States)

    Mattolat, C.; Rothe, S.; Schwellnus, F.; Gottwald, T.; Raeder, S.; Wendt, K.

    2009-03-01

    On-line production facilities for radioactive isotopes nowadays heavily rely on resonance ionization laser ion sources due to their demonstrated unsurpassed efficiency and elemental selectivity. Powerful high repetition rate tunable pulsed dye or Ti:sapphire lasers can be used for this purpose. To counteract limitations of short pulse pump lasers, as needed for dye laser pumping, i.e. copper vapor lasers, which include high maintenance and nevertheless often only imperfect reliability, an all-solid-state Nd:YAG pumped Ti:sapphire laser system has been constructed. This could complement or even replace dye laser systems, eliminating their disadvantages but on the other hand introduce shortcomings on the side of the available wavelength range. Pros and cons of these developments will be discussed.

  13. Plasma diagnostics using laser-excited coupled and transmission ring resonators

    International Nuclear Information System (INIS)

    Haas, R.A.

    1976-01-01

    In this paper a simple two-level laser model is used to investigate the frequency response of coupled-cavity laser interferometers. It is found that under certain circumstances, often satisfied by molecular gas lasers, the frequency response exhibits a resonant behavior. This behavior severely complicates the interpretation of coupled-cavity laser interferometer measurements of rapidly varying plasmas. To circumvent this limitation a new type of laser interferometer plasma diagnostic with significantly improved time response was developed. In this interferometer the plasma is located in one arm of a transmission ring resonator cavity that is excited by an externally positioned laser. Thus, the laser is decoupled from the interferometer cavity and the time response of the interferometer is then limited by the Q of the ring resonator cavity. This improved time response is acquired without loss of spatial resolution, but requires a more sensitive signal detector since the laser is no longer used as a detector as it is in conventional coupled-cavity laser interferometers. Thus, the new technique incorporates the speed of the Mach--Zender interferometer and the sensitivity of the coupled-cavity laser interferometer. The basic operating principles of this type of interferometer have been verified using a CO 2 laser

  14. Injection and laser acceleration of ions based on the resonant surface photoionization

    International Nuclear Information System (INIS)

    Antsiferov, V.V.; Smirnov, G.I.; Telegin, G.G.

    1993-01-01

    The collective effects have been investigated of the injection and acceleration of the ion beams due to the resonant surface photoionization. The considered scheme of the laser accelerator allows to obtain positive ions with relativistic velocities. 11 refs., 2 figs

  15. Nd:YAG (2 omega) pumped dye laser using self-filtering unstable resonator

    CERN Document Server

    Rahimian, K; Hariri, H

    2002-01-01

    A self-filtering unstable resonator with a magnification of M=-3 in a Nd:YAG (2 omega) dye laser has been studied. The dye solution is Rhodamine 6 G in alcohol with the concentration of 5*10 sub - 3 Mol/lit. The spatial intensity distribution of the resonator has been compared has been compared with that of a plane-parallel resonator of equal length. The output energy in both configurations are comparable (20 mu J ,and 26 mu J ,respectively). A significant difference between these two resonators is the laser beam divergence, where beam divergences of 0.77 mrad for the self-filtering unstable resonator and 1.6 mrad for the plane-parallel resonator have been measured. The brightness corresponding to these two resonators are 1.5* 10 sub 1 1 and 2.2* 10 sub 1 0W.cm sub - 2.Sr sub - 1, and the pulse widths are 7 and 17 ns, respectively. These figures show clearly that laser resonator based on the self-filtering unstable resonator design an increase the laser brightness a factor of 10, with a beam divergence of a f...

  16. Manipulating the wavelength-drift of a Tm laser for resonance enhancement in an intra-cavity pumped Ho laser.

    Science.gov (United States)

    Huang, Haizhou; Huang, Jianhong; Liu, Huagang; Li, Jinhui; Lin, Zixiong; Ge, Yan; Dai, Shutao; Deng, Jing; Lin, Wenxiong

    2018-03-05

    We demonstrate an enhancement mechanism and thermal model for intra-cavity pumped lasers, where resonance enhancement in intra-cavity pumped Ho laser was achieved by manipulating the wavelength-drift nature of the Tm laser for the first time. Optical conversion efficiency of 37.5% from an absorbed 785 nm diode laser to a Ho laser was obtained with a maximum output power of 7.51 W at 2122 nm, which is comparable to the conversion efficiency in 1.9 μm LD pumped Ho lasers. Meanwhile, more severe thermal effects in the Ho-doped gain medium than the Tm-doped one at high power operation were verified based on the built thermal model. This work benefits the design or evaluation of intra-cavity pumped lasers, and the resonance enhancement originated from the difference in reabsorption loss between stark levels at the lasing manifolds of quasi-three-level rare-earth ions has great interest to improve the existing intra-cavity pumped lasers or explore novel lasers.

  17. Cyclotron resonant gas breakdown with a 1.22-nm 13CH3F laser

    International Nuclear Information System (INIS)

    Hacker, M.P.; Lax, B.; Metz, R.N.; Temkin, R.J.

    1979-01-01

    Cyclotron-resonant laser-induced gas breakdown has been studied for the first time in the transverse geometry, using 1.222-nm 13 CH 3 F laser radiation propagating perpendicular to the magnetic field axis. The line shape of absorbed laser radiation versus magnetic field near electron cyclotron resonance (87.75 kG) indicates a strong dependence of the line shape on the focused laser intensity. This dependence is not predicted by the standard equilibrium theory of high-frequency gas breakdown in a magnetic field. We have developed an analytic theory to explain the observed line shapes. The theory takes into account the laser propagation characteristics, in particular that there is nonuniform ionization due to strong resonant absorption of the laser radiation in a length comparable to or shorter than that of the laser focal volume. The transverse geometry simplifies the theoretical analysis because the observed line shapes are not significantly affected by Doppler broadening. Extensive data have been obtained on the fraction of laser pulse energy absorbed in the gas breakdown volume as a function of magnetic field, helium gas pressure, and incident laser pulse energy. Good quantitative agreement is obtained between the observed laser pulse absorption line shapes and the nonuniform ionization theory

  18. Design challenges for matrix assisted pulsed laser evaporation and infrared resonant laser evaporation equipment

    Science.gov (United States)

    Greer, James A.

    2011-11-01

    , and evaporation equipment as well. This multilayer feature would certainly benefit the MAPLE process for the growth of multilayer organic materials. Another more recent advancement in thin-film laser deposition is that of Resonant Infra Red Pulsed Laser Deposition (RIRPLD) of polymer materials. This process is more akin to standard PLD but uses tunable lasers with which to select the proper wavelength to couple to vibration bands of a solid polymer, or in some cases a polymer/solvent MAPLE mixture. This technique was developed under a collaboration of researchers at the Naval Research Labs and the Free Electron Laser (FEL) at Vanderbilt University. The wide tuning range of the FEL and its relatively high power make it a very attractive source for RIRPLD. However, the price of such lasers—of order several million dollars in capital costs alone—is very high and well beyond the budgets of most research institutions. Advances in RIRPLD are currently limited due to the scarcity of tunable lasers with sufficient power in the IR range of interest to obtain reasonable deposition rates. Over the past nine years commercial equipment for MAPLE has been on the market and new lasers are being developed that may significantly improve MAPLE and RIRPLD capabilities. Examples of basic single-target MAPLE equipment, as well as multiple target MAPLE systems are described. Discussion of current lasers for MAPLE and RIRPLD are given. Finally, even though these processes have been around for a significant amount of time there are still many unknowns associated with these techniques that still should be explored before these processes can be used for production of useful products. Some of these issues which need to be addressed will be discussed.

  19. Highly scalable, resonantly cladding-pumped, Er-doped fiber laser with record efficiency.

    Science.gov (United States)

    Dubinskii, M; Zhang, J; Ter-Mikirtychev, V

    2009-05-15

    We report the performance of a resonantly cladding-pumped, Yb-free, Er-doped fiber laser. We believe this is the first reported resonantly cladding-pumped fiber-Bragg-grating-based, Er-doped, large-mode-area (LMA) fiber laser. The laser, pumped by fiber-coupled InGaAsP/InP laser diode modules at 1,532.5 nm, delivers approximately 48 W of cw output at 1,590 nm. It is believed to be the highest power ever reported from a Yb-free Er-doped LMA fiber. This fully integrated laser also has the optical-to-optical efficiency of approximately 57%, to the best of our knowledge, the highest efficiency reported for cladding-pumped unidirectionally emitting Er-doped laser.

  20. Time-resolved resonance fluorescence spectroscopy for study of chemical reactions in laser-induced plasmas.

    Science.gov (United States)

    Liu, Lei; Deng, Leimin; Fan, Lisha; Huang, Xi; Lu, Yao; Shen, Xiaokang; Jiang, Lan; Silvain, Jean-François; Lu, Yongfeng

    2017-10-30

    Identification of chemical intermediates and study of chemical reaction pathways and mechanisms in laser-induced plasmas are important for laser-ablated applications. Laser-induced breakdown spectroscopy (LIBS), as a promising spectroscopic technique, is efficient for elemental analyses but can only provide limited information about chemical products in laser-induced plasmas. In this work, time-resolved resonance fluorescence spectroscopy was studied as a promising tool for the study of chemical reactions in laser-induced plasmas. Resonance fluorescence excitation of diatomic aluminum monoxide (AlO) and triatomic dialuminum monoxide (Al 2 O) was used to identify these chemical intermediates. Time-resolved fluorescence spectra of AlO and Al 2 O were used to observe the temporal evolution in laser-induced Al plasmas and to study their formation in the Al-O 2 chemistry in air.

  1. Effect of polarization and focusing on laser pulse driven auto-resonant particle acceleration

    International Nuclear Information System (INIS)

    Sagar, Vikram; Sengupta, Sudip; Kaw, Predhiman

    2014-01-01

    The effect of laser polarization and focusing is theoretically studied on the final energy gain of a particle in the Auto-resonant acceleration scheme using a finite duration laser pulse with Gaussian shaped temporal envelope. The exact expressions for dynamical variables viz. position, momentum, and energy are obtained by analytically solving the relativistic equation of motion describing particle dynamics in the combined field of an elliptically polarized finite duration pulse and homogeneous static axial magnetic field. From the solutions, it is shown that for a given set of laser parameters viz. intensity and pulse length along with static magnetic field, the energy gain by a positively charged particle is maximum for a right circularly polarized laser pulse. Further, a new scheme is proposed for particle acceleration by subjecting it to the combined field of a focused finite duration laser pulse and static axial magnetic field. In this scheme, the particle is initially accelerated by the focused laser field, which drives the non-resonant particle to second stage of acceleration by cyclotron Auto-resonance. The new scheme is found to be efficient over two individual schemes, i.e., auto-resonant acceleration and direct acceleration by focused laser field, as significant particle acceleration can be achieved at one order lesser values of static axial magnetic field and laser intensity

  2. Photonic crystal Fano resonances for realizing optical switches, lasers and non-reciprocal elements

    DEFF Research Database (Denmark)

    Bekele, Dagmawi Alemayehu; Yu, Yi; Hu, Hao

    2017-01-01

    structure in combination with cavity-enhanced nonlinearity can be used to realize non-reciprocal transmission at ultra-low power and with large bandwidth. A novel type of laser structure, denoted a Fano laser, is discussed in which one of the mirrors is based on a Fano resonance. Finally, the design...

  3. Resonant laser mass spectrometry for environmental and industrial chemical trace analysis

    International Nuclear Information System (INIS)

    Boesl, Ulrich; Rink, Joerg; Distelrath, Volker; Pueffel, Peter

    2001-01-01

    A promising new method for pollutant trace analysis is resonant laser mass spectrometry. It combines selectivity, sensitivity, and speed of measurement. In this paper, two examples of application are presented: exhaust analysis of combustion engines and analysis of polycylcic aromatic compounds in soil samples. The sensitivity of small, mobile instruments is discussed as well as alternative laser-based techniques in the case formation of cations by nanosecond lasers is improbable

  4. Bistable laser device with multiple coupled active vertical-cavity resonators

    Science.gov (United States)

    Fischer, Arthur J.; Choquette, Kent D.; Chow, Weng W.

    2003-08-19

    A new class of bistable coupled-resonator vertical-cavity semiconductor laser devices has been developed. These bistable laser devices can be switched, either electrically or optically, between lasing and non-lasing states. A switching signal with a power of a fraction of a milliwatt can change the laser output of such a device by a factor of a hundred, thereby enabling a range of optical switching and data encoding applications.

  5. Two-step resonance ionization spectroscopy of Na atomic beam using cw and pulsed lasers

    International Nuclear Information System (INIS)

    Katsuragawa, H.; Minowa, T.; Shimazu, M.

    1988-01-01

    Two-step photoionization of sodium atomic beam has been carried out using a cw and a pulsed dye lasers. Sodium ions have been detected by a time of flight method in order to reduce background noise. With a proper power of the pulsed dye laser the sodium atomic beam has been irradiated by a resonant cw dye laser. The density of the sodium atomic beam is estimated to be 10 3 cm -3 at the ionization area. (author)

  6. Quasibound levels and shape resonances of 39K2(B 1Pi/sub u/) crossed laser-molecular beam studies and analytical interpretation

    International Nuclear Information System (INIS)

    Heinze, J.; Kowalczyk, P.; Engelke, F.

    1988-01-01

    Quasibound levels and shape resonances in the (B 1 Pi/sub u/ -X 1 Σ + /sub g/) band system of 39 K 2 have been recorded by crossed laser-molecular beam techniques. Using optical--optical double resonance, individual rovibrational levels (v'' = 15--18, J'' = 3--25) of the K 2 state are prepared by Franck--Condon pumping (FCP) in a supersonic nozzle beam. Excitation into quasibound levels below and above the (B 1 Pi/sub u/) state barrier is detected as molecular and atomic (K4 2 P 3 /sub // 2 →4 2 S 1 /sub // 2 only) fluorescence. The resonance transition frequencies and shapes are measured and the results are used (a) to determine the scattering resonance energies, widths, and lifetimes; (b) to compare them with values obtained by a ''maximum internal amplitude'' approach [R. J. LeRoy and R. B. Bernstein, J. Chem. Phys. 54, 5114 (1971)]; and (c) to check the agreement with exact calculations of the B state potential using the ''inverted perturbation approach (IPA).'' The bound and quasibound part of the B 1 Pi/sub u/ state including the locus (R = 8.08 +- 0.05 A) of the barrier maximum (298 +- 8 cm -1 above the adiabatic dissociation limit) is found in excellent agreement with previous results. The shape resonances are not highly sensitive to the long-range interatomic forces, here the repulsive dipole--dipole resonance interaction

  7. A three-dimensional model for calculating the micro disk laser resonant-modes

    International Nuclear Information System (INIS)

    Sabetjoo, H.; Bahrampor, A.; Farrahi-Moghaddam, R.

    2006-01-01

    In this article, a semi-analytical model for theoretical analysis of micro disk lasers is presented. Using this model, the necessary conditions for the existence of loss less and low-loss modes of micro-resonators are obtained. The resonance frequency of the resonant modes and also the attenuation of low-loss modes are calculated. By comparing the results with results of finite difference method, their validity is certified.

  8. Resonator design and performance estimation for a space-based laser transmitter

    Science.gov (United States)

    Agrawal, Lalita; Bhardwaj, Atul; Pal, Suranjan; Kamalakar, J. A.

    2006-12-01

    Development of a laser transmitter for space applications is a highly challenging task. The laser must be rugged, reliable, lightweight, compact and energy efficient. Most of these features are inherently achieved by diode pumping of solid state lasers. Overall system reliability can further be improved by appropriate optical design of the laser resonator besides selection of suitable electro-optical and opto-mechanical components. This paper presents the design details and the theoretically estimated performance of a crossed-porro prism based, folded Z-shaped laser resonator. A symmetrically pumped Nd: YAG laser rod of 3 mm diameter and 60 mm length is placed in the gain arm with total input peak power of 1800 W from laser diode arrays. Electro-optical Q-switching is achieved through a combination of a polarizer, a fractional waveplate and LiNbO 3 Q-switch crystal (9 x 9 x 25 mm) placed in the feedback arm. Polarization coupled output is obtained by optimizing azimuth angle of quarter wave plate placed in the gain arm. Theoretical estimation of laser output energy and pulse width has been carried out by varying input power levels and resonator length to analyse the performance tolerances. The designed system is capable of meeting the objective of generating laser pulses of 10 ns duration and 30 mJ energy @ 10 Hz.

  9. A high-power diode-laser-pumped CW Nd:YAG laser using a stable-unstable resonator

    International Nuclear Information System (INIS)

    Mudge, M.; Ostermeyer, P.; Veitch, J.; Munch, J.; Hamilton, M.W.

    2000-01-01

    Full text: The design and operation of a power-scalable diode-laser-pumped CW Nd:YAG zigzag slab laser that uses a stable-unstable resonator with a graded reflectivity mirror as an output coupler is described. We demonstrate control of the thermal lens strength in the unstable plane and weak thermal lensing in the stable plane that is independent of pump power, vital for efficient scalability. This enabled CW operation of the stable-unstable resonator with excellent near- and far-field beam quality

  10. Stochastic resonance in a single-mode laser driven by frequency modulated signal and coloured noises

    Institute of Scientific and Technical Information of China (English)

    Jin Guo-Xiang; Zhang Liang-Ying; Cao Li

    2009-01-01

    By adding frequency modulated signals to the intensity equation of gain-noise model of the single-mode laser driven by two coloured noises which are correlated, this paper uses the linear approximation method to calculate the power spectrum and signal-to-noise ratio (SNR) of the laser intensity. The results show that the SNR appears typical stochastic resonance with the variation of intensity of the pump noise and quantum noise. As the amplitude of a modulated signal has effects on the SNR, it shows suppression, monotone increasing, stochastic resonance, and multiple stochastic resonance with the variation of the frequency of a carrier signal and modulated signal.

  11. Performance of terahertz metamaterials as high-sensitivity sensor

    Science.gov (United States)

    He, Yanan; Zhang, Bo; Shen, Jingling

    2017-09-01

    A high-sensitivity sensor based on the resonant transmission characteristics of terahertz (THz) metamaterials was investigated, with the proposal and fabrication of rectangular bar arrays of THz metamaterials exhibiting a period of 180 μm on a 25 μm thick flexible polyimide. Varying the size of the metamaterial structure revealed that the length of the rectangular unit modulated the resonant frequency, which was verified by both experiment and simulation. The sensing characteristics upon varying the surrounding media in the sample were tested by simulation and experiment. Changing the surrounding medium from that of air to that of alcohol or oil produced resonant frequency redshifts of 80 GHz or 150 GHz, respectively, which indicates that the sensor possessed a high sensitivity of 667 GHz per unit of refractive index. Finally, the influence of the sample substrate thickness on the sensor sensitivity was investigated by simulation. It may be a reference for future sensor design.

  12. Continuous-wave singly resonant optical parametric oscillator placed inside a ring laser

    DEFF Research Database (Denmark)

    Abitan, Haim; Buchhave, Preben

    2003-01-01

    A cw singly resonant optical parametric oscillator (SRO) was built and placed inside the cavity of a ring laser. The system consists of a diode-end-pumped Nd:YVO4 ring laser with intracavity periodically poled lithium niobate as the nonlinear gain medium of the SRO. When the laser was operated...... in a unidirectional mode, we obtained more than 520 mW of signal power in one beam. When the laser was operated in a bidirectional mode, we obtained 600 mW of signal power (300 mW in two separate beams). The power and the spectral features of the laser in the unidirectional and bidirectional modes were measured while...... the laser was coupled with the SRO. The results show that it is preferable to couple a SRO with a unidirectional ring laser....

  13. Developing laser ablation in an electron cyclotron resonance ion source for actinide detection with AMS

    Energy Technology Data Exchange (ETDEWEB)

    Bauder, W. [Argonne National Laboratory, Physics Division, 9600 S. Cass Ave, Lemont, IL 60439 (United States); University of Notre Dame, Nuclear Science Laboratory, 124 Nieuwland Science Hall, Notre Dame, IN 46556 (United States); Pardo, R.C.; Kondev, F.G.; Kondrashev, S.; Nair, C.; Nusair, O. [Argonne National Laboratory, Physics Division, 9600 S. Cass Ave, Lemont, IL 60439 (United States); Palchan, T. [Hebrew University, Racah Institute of Physics, Jerusalem 91904 (Israel); Scott, R.; Seweryniak, D.; Vondrasek, R. [Argonne National Laboratory, Physics Division, 9600 S. Cass Ave, Lemont, IL 60439 (United States); Collon, P. [University of Notre Dame, Nuclear Science Laboratory, 124 Nieuwland Science Hall, Notre Dame, IN 46556 (United States); Paul, M. [Hebrew University, Racah Institute of Physics, Jerusalem 91904 (Israel)

    2015-10-15

    A laser ablation material injection system has been developed at the ATLAS electron cyclotron resonance (ECR) ion source for use in accelerator mass spectrometry experiments. Beam production with laser ablation initially suffered from instabilities due to fluctuations in laser energy and cratering on the sample surface by the laser. However, these instabilities were rectified by applying feedback correction for the laser energy and rastering the laser across the sample surface. An initial experiment successfully produced and accelerated low intensity actinide beams with up to 1000 counts per second. With continued development, laser ablation shows promise as an alternative material injection scheme for ECR ion sources and may help substantially reduce cross talk in the source.

  14. Resonance ionization laser ion sources for on-line isotope separators (invited)

    International Nuclear Information System (INIS)

    Marsh, B. A.

    2014-01-01

    A Resonance Ionization Laser Ion Source (RILIS) is today considered an essential component of the majority of Isotope Separator On Line (ISOL) facilities; there are seven laser ion sources currently operational at ISOL facilities worldwide and several more are under development. The ionization mechanism is a highly element selective multi-step resonance photo-absorption process that requires a specifically tailored laser configuration for each chemical element. For some isotopes, isomer selective ionization may even be achieved by exploiting the differences in hyperfine structures of an atomic transition for different nuclear spin states. For many radioactive ion beam experiments, laser resonance ionization is the only means of achieving an acceptable level of beam purity without compromising isotope yield. Furthermore, by performing element selection at the location of the ion source, the propagation of unwanted radioactivity downstream of the target assembly is reduced. Whilst advances in laser technology have improved the performance and reliability of laser ion sources and broadened the range of suitable commercially available laser systems, many recent developments have focused rather on the laser/atom interaction region in the quest for increased selectivity and/or improved spectral resolution. Much of the progress in this area has been achieved by decoupling the laser ionization from competing ionization processes through the use of a laser/atom interaction region that is physically separated from the target chamber. A new application of gas catcher laser ion source technology promises to expand the capabilities of projectile fragmentation facilities through the conversion of otherwise discarded reaction fragments into high-purity low-energy ion beams. A summary of recent RILIS developments and the current status of laser ion sources worldwide is presented

  15. Emergence of resonant mode-locking via delayed feedback in quantum dot semiconductor lasers.

    Science.gov (United States)

    Tykalewicz, B; Goulding, D; Hegarty, S P; Huyet, G; Erneux, T; Kelleher, B; Viktorov, E A

    2016-02-22

    With conventional semiconductor lasers undergoing external optical feedback, a chaotic output is typically observed even for moderate levels of the feedback strength. In this paper we examine single mode quantum dot lasers under strong optical feedback conditions and show that an entirely new dynamical regime is found consisting of spontaneous mode-locking via a resonance between the relaxation oscillation frequency and the external cavity repetition rate. Experimental observations are supported by detailed numerical simulations of rate equations appropriate for this laser type. The phenomenon constitutes an entirely new mode-locking mechanism in semiconductor lasers.

  16. Polariton condensation, superradiance and difference combination parametric resonance in mode-locked laser

    Science.gov (United States)

    Bagayev, S. N.; Arkhipov, R. M.; Arkhipov, M. V.; Egorov, V. S.; Chekhonin, I. A.; Chekhonin, M. A.

    2017-11-01

    The generation of the ring mode-locked laser containing resonant absorption medium in the cavity was investigated. It is shown that near the strong resonant absorption lines a condensation of polaritons arises. Intensive radiation looks like as superradiance in a medium without population inversion. We studied theoretically the microscopic mechanism of these phenomena. It was shown that in this system in absorbing medium a strong self-induced difference combination parametric resonance exists. Superradiance on polaritonic modes in the absorbing medium are due to the emergence of light-induced resonant polarization as a result of fast periodic nonadiabatic quantum jumps in the absorber.

  17. Single-frequency, fully integrated, miniature DPSS laser based on monolithic resonator

    Science.gov (United States)

    Dudzik, G.; Sotor, J.; Krzempek, K.; Soboń, G.; Abramski, K. M.

    2014-02-01

    We present a single frequency, stable, narrow linewidth, miniature laser sources operating at 532 nm (or 1064 nm) based on a monolithic resonators. Such resonators utilize birefringent filters formed by YVO4 beam displacer and KTP or YVO4 crystals to force single frequency operation at 532 nm or 1064 nm, respectively. In both configurations Nd:YVO4 gain crystal is used. The resonators dimensions are 1x1x10.5 mm3 and 1x1x8.5 mm3 for green and infrared configurations, respectively. Presented laser devices, with total dimensions of 40x52x120 mm3, are fully equipped with driving electronics, pump diode, optical and mechanical components. The highly integrated (36x15x65 mm3) low noise driving electronics with implemented digital PID controller was designed. It provides pump current and resonator temperature stability of ±30 μA@650 mA and ±0,003ºC, respectively. The laser parameters can be set and monitored via the USB interface by external application. The developed laser construction is universal. Hence, the other wavelengths can be obtained only by replacing the monolithic resonator. The optical output powers in single frequency regime was at the level of 42 mW@532 nm and 0.5 W@1064 nm with the long-term fluctuations of ±0.85 %. The linewidth and the passive frequency stability under the free running conditions were Δν < 100 kHz and 3ṡ10-9@1 s integration time, respectively. The total electrical power supply consumption of laser module was only 4 W. Presented compact, single frequency laser operating at 532 nm and 1064 nm may be used as an excellent source for laser vibrometry, interferometry or seed laser for fiber amplifiers.

  18. XeCl excimer laser with new prism resonator configurations and its performance characteristics

    Energy Technology Data Exchange (ETDEWEB)

    Benerji, N. S., E-mail: nsb@rrcat.gov.in, E-mail: bsingh@rrcat.gov.in; Singh, A.; Varshnay, N.; Singh, Bijendra, E-mail: nsb@rrcat.gov.in, E-mail: bsingh@rrcat.gov.in [Excimer Laser Section, LMPD, Raja Ramanna Center for Advanced Technology, Indore 452013 (India)

    2015-07-15

    New resonator cavity configurations, namely, the prism resonator and unstable prism resonator, are demonstrated for the first time in an excimer (XeCl) laser with interesting and novel results. High misalignment tolerance ∼50 mrad is achieved with considerably reduced beam divergence of less than ∼1 mrad without reduction in output power capabilities of the laser. The misalignment tolerance of ∼50 mrad is a dramatic improvement of ∼25 times compared to ∼2 mrad normally observed in standard excimer laser with plane-plane cavity. Increase in depth of focus from 3 mm to 5.5 mm was also achieved in case of prism resonator configuration with an improvement of about 60%. Unstable prism resonator configuration is demonstrated here in this paper with further reduction in beam divergence to about 0.5 mrad using plano-convex lens as output coupler. The misalignment tolerance in case of unstable prism resonator was retained at about 30 mrad which is a high value compared to standard unstable resonators. The output beam spot was completely filled with flat-top profile with prism resonator configurations, which is desired for various material processing applications. Focusing properties and beam divergence in case of prism resonator have been investigated using SEM (scanning electron microscope) images. SEM images of the focused spot size (∼20 μm holes) on metal sheet indicate beam divergence of about 0.05 mrad which is about 1.5 times diffraction limit. Energy contained in this angle is thus sufficient for micro-machining applications. Clean and sharp edges of the micro-holes show high pointing stability with multiple shot exposures. Such characteristics of the excimer laser system will be extremely useful in micro-machining and other field applications.

  19. Modeling and simulation of two-step resonance ionization processes using CW and pulsed lasers

    CERN Document Server

    de Groote, Ruben; Flanagan, Kieran

    This thesis derives and discusses equations that describe the evolution of atomic systems subjected to two monochromatic and coherent radiation fields and treats both continuous and temporally pulsed irradiation. This theoretical description is de- veloped mainly to understand the influence of the photon field intensities on experimental ionization spectra. The primary ap- plication of this theoretical framework is on methods that rely on resonant laser excitation and non-resonant laser ionization to extract information on the hyperfine structure of atomic systems. In particular, qualitative and quantitative discussions on the laser-related changes in hyperfine splitting extracted from ion- ization spectra are presented. Also, a method for increasing the resolution of resonance ionization techniques (potentially up un- til the natural linewidth of the electronic transitions) is discussed and theoretically justified. Both topics are illustrated with exper- imental data.

  20. Dynamics of moving interacting atoms in a laser radiation field and optical size resonances

    International Nuclear Information System (INIS)

    Gadomskii, O.N.; Glukhov, A.G.

    2005-01-01

    The forces acting on interacting moving atoms exposed to resonant laser radiation are calculated. It is shown that the forces acting on the atoms include the radiation pressure forces as well as the external and internal bias forces. The dependences of the forces on the atomic spacing, polarization, and laser radiation frequency are given. It is found that the internal bias force associated with the interaction of atomic dipoles via the reemitted field may play an important role in the dynamics of dense atomic ensembles in a light field. It is shown that optical size resonances appear in the system of interacting atoms at frequencies differing substantially from transition frequencies in the spectrum of atoms. It is noted that optical size resonances as well as the Doppler frequency shift in the spectrum of interacting atoms play a significant role in the processes of laser-radiation-controlled motion of the atoms

  1. Resonantly diode-pumped continuous-wave and Q-switched Er:YAG laser at 1645 nm.

    Science.gov (United States)

    Chang, N W H; Simakov, N; Hosken, D J; Munch, J; Ottaway, D J; Veitch, P J

    2010-06-21

    We describe an efficient Er:YAG laser that is resonantly pumped using continuous-wave (CW) laser diodes at 1470 nm. For CW lasing, it emits 6.1 W at 1645 nm with a slope efficiency of 36%, the highest efficiency reported for an Er:YAG laser that is pumped in this manner. In Q-switched operation, the laser produces diffraction-limited pulses with an average power of 2.5 W at 2 kHz PRF. To our knowledge this is the first Q-switched Er:YAG laser resonantly pumped by CW laser diodes.

  2. Resonance ionization in a gas cell: a feasibility study for a laser ion source

    International Nuclear Information System (INIS)

    Qamhieh, Z.N.; Vandeweert, E.; Silverans, R.E.; Duppen, P. van; Huyse, M.; Vermeeren, L.

    1992-01-01

    A laser ion source based on resonance photo-ionization in a gas cell is proposed. The gas cell, filled with helium, consists of a target chamber in which the recoil products are stopped and neutralized, and an ionization chamber where the atoms of interest are selectively ionized by the laser light. The extraction of the ions from the ionization chamber through the exit hole-skimmer setup is similar to the ion-guide system. The conditions to obtain an optimal system are given. The results of a two-step one-laser resonance photo-ionization of nickel and the first results of laser ionization in a helium buffer gas cell are presented. (orig.)

  3. Nonlinear resonance phenomena of a doped fibre laser under cavity ...

    Indian Academy of Sciences (India)

    quence and other routes to chaos, generalized multistability and crisis. But, doped ... of chaos and synchronization of coupled chaotic lasers (for communication with a ... The two basic issues in focus here for the nonlinear dynamical studies.

  4. Resonance-enhanced laser-induced plasma spectroscopy for sensitive elemental analysis: Elucidation of enhancement mechanisms

    International Nuclear Information System (INIS)

    Lui, S.L.; Cheung, N.H.

    2002-01-01

    When performing laser-induced plasma spectroscopy for elemental analysis, the analyte signal-to-noise ratio increased from four to over fifty if the plume was reheated by a dye laser pulse tuned to resonant absorption. Time-resolved studies showed that the enhancement was not due to resonance photoionization. Rather, efficient and controlled rekindling of a larger plume volume was the key mechanism. The signal-to-noise ratio further increased to over a hundred if the atmosphere was replaced by a low-pressure heavy inert gas. The ambient gas helped confine and thermally insulate the expanding vapor

  5. Radiation reaction effect on laser driven auto-resonant particle acceleration

    International Nuclear Information System (INIS)

    Sagar, Vikram; Sengupta, Sudip; Kaw, P. K.

    2015-01-01

    The effects of radiation reaction force on laser driven auto-resonant particle acceleration scheme are studied using Landau-Lifshitz equation of motion. These studies are carried out for both linear and circularly polarized laser fields in the presence of static axial magnetic field. From the parametric study, a radiation reaction dominated region has been identified in which the particle dynamics is greatly effected by this force. In the radiation reaction dominated region, the two significant effects on particle dynamics are seen, viz., (1) saturation in energy gain by the initially resonant particle and (2) net energy gain by an initially non-resonant particle which is caused due to resonance broadening. It has been further shown that with the relaxation of resonance condition and with optimum choice of parameters, this scheme may become competitive with the other present-day laser driven particle acceleration schemes. The quantum corrections to the Landau-Lifshitz equation of motion have also been taken into account. The difference in the energy gain estimates of the particle by the quantum corrected and classical Landau-Lifshitz equation is found to be insignificant for the present day as well as upcoming laser facilities

  6. The laser elevator - Momentum transfer using an optical resonator

    Science.gov (United States)

    Meyer, Thomas R.; Mckay, Christopher P.; Mckenna, Paul M.

    1987-01-01

    In a conventional laser lightsail system the payload is propelled by the momentum imparted to it by the reflection of a laser beam without the use of any propellant. Because of the unfavorable relationship between energy and momentum in a light beam, these systems are very inefficient. The efficiency can be greatly improved, in principle, if the photons that impact the payload mirror are returned to the source and then redirected back toward the payload again. This system, which recirculates the laser beam, is defined as the 'laser elevator'. The gain of the laser elevator over conventional lightsails depends on the number of times the beam is recycled which is limited by the reflectance of the mirrors used, any losses in the transmission of the beam, and diffraction. Due to the increase pathlength of the folded beam, diffraction losses occur at smaller separations of the payload and the source mirror than for conventional lightsail system. The laser elevator has potential applications in launching to low earth orbit, orbital transfer, and rapid interplanetary delivery of small payloads.

  7. Calculation of a CO sub 2 gasdynamic laser with selective thermal excitation and an unstable resonator

    Energy Technology Data Exchange (ETDEWEB)

    Kuz' min, A.I.; Lavrov, A.V.; Chernysheva, N.V. (Leningradskii Gosudarstvennyi Universitet, Leningrad (USSR))

    1989-03-01

    The problem of calculating an unstable telescopic resonator for a CO{sub 2} gasdynamic laser with selective thermal excitation is studied. Parabolized Navier-Stokes equations and equations of field propagation in the resonator are used to describe the GDL in the geometric optic approximation. The efficiency is studied as a function of the magnification factor and of the distance between the mirrors. 19 refs.

  8. Magnetic resonance thermometry for monitoring photothermal effects of interstitial laser irradiation

    Science.gov (United States)

    Goddard, Jessica; Jose, Jessnie; Figueroa, Daniel; Le, Kelvin; Liu, Hong; Nordquist, Robert E.; Hode, Tomas; Chen, Wei R.

    2012-03-01

    Selective photothermal interaction using dye-assisted non-invasive laser irradiation has limitations when treating deeper tumors or when the overlying skin is heavily pigmented. We developed an interstitial laser irradiation method to induce the desired photothermal effects. An 805-nm near-infrared laser with a cylindrical diffuser was used to treat rat mammary tumors by placing the active tip of the fiber inside the target tumors. Three different power settings (1.0 to 1.5 watts) were applied to treat animal tumors with an irradiation duration of 10 minutes. The temperature distributions of the treated tumors were measured by a 7.1-Tesla magnetic resonance imager using proton resonance frequency (PRF) method. Three-dimensional temperature profiles were reconstructed and assessed using PRF. This is the first time a 7.1-Tesla magnetic resonance imager has been used to monitor interstitial laser irradiation via PRF. This study provides a basic understanding of the photothermal interaction needed to control the thermal damage inside tumor using interstitial laser irradiation. It also shows that PRF can be used effectively in monitoring photothermal interaction. Our long-term goal is to develop a PRF-guided laser therapy for cancer treatment.

  9. Double threshold behavior in a resonance-controlled ZnO random laser

    Directory of Open Access Journals (Sweden)

    Ryo Niyuki

    2017-03-01

    Full Text Available We observed unusual lasing characteristics, such as double thresholds and blue-shift of lasing peak, in a resonance-controlled ZnO random laser. From the analysis of lasing threshold carrier density, we found that the lasing at 1st and 2nd thresholds possibly arises from different mechanisms; the lasing at 1st threshold involves exciton recombination, whereas the lasing at 2nd threshold is caused by electron-hole plasma recombination, which is the typical origin of conventional random lasers. These phenomena are very similar to the transition from polariton lasing to photon lasing observed in a well-defined cavity laser.

  10. Diode laser based resonance ionization mass spectrometry for spectroscopy and trace analysis of uranium isotopes

    International Nuclear Information System (INIS)

    Hakimi, Amin

    2013-01-01

    In this doctoral thesis, the upgrade and optimization of a diode laser system for high-resolution resonance ionization mass spectrometry is described. A frequency-control system, based on a double-interferometric approach, allowing for absolute stabilization down to 1 MHz as well as frequency detunings of several GHz within a second for up to three lasers in parallel was optimized. This laser system was used for spectroscopic studies on uranium isotopes, yielding precise and unambiguous level energies, total angular momenta, hyperfine constants and isotope shifts. Furthermore, an efficient excitation scheme which can be operated with commercial diode lasers was developed. The performance of the complete laser mass spectrometer was optimized and characterized for the ultra-trace analysis of the uranium isotope 236 U, which serves as a neutron flux dosimeter and tracer for radioactive anthropogenic contaminations in the environment. Using synthetic samples, an isotope selectivity of ( 236 U)/( 238 U) = 4.5(1.5) . 10 -9 was demonstrated.

  11. Off-resonance plasmonic enhanced femtosecond laser optoporation and transfection of cancer cells.

    Science.gov (United States)

    Baumgart, Judith; Humbert, Laure; Boulais, Étienne; Lachaine, Rémi; Lebrun, Jean-Jaques; Meunier, Michel

    2012-03-01

    A femtosecond laser based transfection method using off-resonance plasmonic gold nanoparticles is described. For human cancer melanoma cells, the treatment leads to a very high perforation rate of 70%, transfection efficiency three times higher than for conventional lipofection, and very low toxicity (transfection for skin cancer treatment. Copyright © 2011 Elsevier Ltd. All rights reserved.

  12. Anisotropy in semipolar InGaN laser diodes: Consequences for resonator design and facet formation

    Energy Technology Data Exchange (ETDEWEB)

    Rass, Jens; Vogt, Patrick [Technische Universitaet Berlin (Germany). Institute of Solid State Physics; Wernicke, Tim; John, Wilfred; Einfeldt, Sven; Weyers, Markus [Ferdinand-Braun-Institut fuer Hoechstfrequenztechnik, Berlin (Germany); Kneissl, Michael [Technische Universitaet Berlin (Germany). Institute of Solid State Physics; Ferdinand-Braun-Institut fuer Hoechstfrequenztechnik, Berlin (Germany)

    2010-07-01

    For InAlGaN-based light emitting devices on nonpolar and semipolar substrate orientations the polarization fields can be reduced. Birefringence and gain anisotropy influence the optical modes of semipolar separate confinement hetero structures. We have investigated the threshold for amplified spontaneous emission and the optical polarization state of the eigenmodes for laser resonators with different orientations on various semipolar and nonpolar substrates. We found that semipolar resonators along the projection of the c-axis onto the surface have a lower threshold and the light is TE-polarized. Nonpolar resonators perpendicular to the c-axis on the other hand have elevated thresholds and hence a lower gain as well as a tilted linear optical polarization with the electric field nearly parallel to the c-axis of the crystal. In order to obtain devices with low threshold and maximum performance, laser resonators on semipolar substrates have to be oriented along the semipolar orientation, posing a challenge for the fabrication of laser facets. Technologies such as laser assisted cleaving, chemical dry etching and wet chemical post processing are presented and their suitability for the generation of smooth vertical facets is discussed.

  13. Focusing effects of a laser beam in the non resonant MPI of gases

    International Nuclear Information System (INIS)

    Baravian, G.; Sultan, G.

    1984-09-01

    The authors give a method to interpret correctly the multiphoton ionization in the case of no resonance and saturation. The calculation model is applied to hydrogen to calculate the ion production related to the intensity of laser pulse. Different applications and methods are given. The six-photon ionization cross-section of the krypton is calculated [fr

  14. Laser resonance ionization for ultra-trace analysis on long-lived ...

    Indian Academy of Sciences (India)

    for producing pure beams of short-lived isotopes at on-line facilities. .... mental design is to develop a compact table-top RIS experiment which allows for. 1058 ... partial beams which are merged by dichroic mirrors and polarization beam splitter ... A quasi-cw 35 W CO2 laser is used for efficient non-resonant ionization of.

  15. Laser scattering off of alpha particle cyclotron harmonic resonances: Annual performance report

    International Nuclear Information System (INIS)

    Aamodt, R.E.

    1988-01-01

    The active probing of burning plasmas to quantitatively determine high energy alpha particle characteristics is the main purpose of the laser and gyroton scattering program. Progress to date includes a systematic evaluation of homogeneous results, analytical study of alpha particle harmonic resonances, and investigations of finite size detection systems

  16. Monolithic integration of a resonant tunneling diode and a quantum well semiconductor laser

    Science.gov (United States)

    Grave, I.; Kan, S. C.; Griffel, G.; Wu, S. W.; Sa'Ar, A.

    1991-01-01

    A monolithic integration of a double barrier AlAs/GaAs resonant tunneling diode and a GaAs/AlGaAs quantum well laser is reported. Negative differential resistance and negative differential optical response are observed at room temperature. The device displays bistable electrical and optical characteristics which are voltage controlled. Operation as a two-state optical memory is demonstrated.

  17. Resonance fluorescence spectra of a three-level atom driven by two strong laser fields

    International Nuclear Information System (INIS)

    Peng Jinsheng.

    1986-12-01

    The resonance fluorescence of a three-level atom interacted with two high-power laser fields is investigated in strong field approximation. The fluorescence distribution is obtained by means of the theory of dressing transformation. (author). 15 refs, 2 figs

  18. Surface plasmon resonance assisted rapid laser joining of glass

    Energy Technology Data Exchange (ETDEWEB)

    Zolotovskaya, Svetlana A.; Tang, Guang; Abdolvand, Amin, E-mail: a.abdolvand@dundee.ac.uk [School of Engineering, Physics and Mathematics, University of Dundee, Dundee DD1 4HN (United Kingdom); Wang, Zengbo [School of Electronic Engineering, Bangor University, Bangor LL57 1UT (United Kingdom)

    2014-08-25

    Rapid and strong joining of clear glass to glass containing randomly distributed embedded spherical silver nanoparticles upon nanosecond pulsed laser irradiation (∼40 ns and repetition rate of 100 kHz) at 532 nm is demonstrated. The embedded silver nanoparticles were ∼30–40 nm in diameter, contained in a thin surface layer of ∼10 μm. A joint strength of 12.5 MPa was achieved for a laser fluence of only ∼0.13 J/cm{sup 2} and scanning speed of 10 mm/s. The bonding mechanism is discussed in terms of absorption of the laser energy by nanoparticles and the transfer of the accumulated localised heat to the surrounding glass leading to the local melting and formation of a strong bond. The presented technique is scalable and overcomes a number of serious challenges for a widespread adoption of laser-assisted rapid joining of glass substrates, enabling applications in the manufacture of microelectronic devices, sensors, micro-fluidic, and medical devices.

  19. Holographic Resonant Laser Printing of Metasurfaces Using Plasmonic Template

    DEFF Research Database (Denmark)

    Carstensen, Marcus S.; Zhu, Xiaolong; Iyore, Oseze Esther

    2018-01-01

    Laser printing with a spatial light modulator (SLM) has several advantages over conventional raster-writing and dot-matrix display (DMD) writing: multiple pixel exposure, high power endurance and existing software for computer generated holograms (CGH). We present a technique for the design...

  20. Resonance-enhanced laser-induced plasma spectroscopy: ambient gas effects

    International Nuclear Information System (INIS)

    Lui, S.L.; Cheung, N.H.

    2003-01-01

    When performing laser-induced plasma spectroscopy for elemental analysis, the sensitivity could be significantly enhanced if the plume was resonantly rekindled by a dye laser pulse. The extent of the enhancement was found to depend on the ambient gas. Air, nitrogen, helium, argon and xenon at pressures ranging from vacuum to 1 bar were investigated. In vacuum, the analyte signal was boosted because of reduced cooling, but it soon decayed as the plume freely expanded. By choosing the right ambient gas at the right pressure, the expanding plume could be confined as well as thermally insulated to maximize the analyte signal. For instance, an ambient of 13 mbar xenon yielded a signal-to-noise ratio of 110. That ratio was 53 when the pellet was ablated in air, and decreased further to 5 if the dye laser was tuned off resonance

  1. Improving the Selectivity of the ISOLDE Resonance Ionization Laser Ion Source and In-Source Laser Spectroscopy of Polonium

    CERN Document Server

    Fink, Daniel Andreas; Jochim, Selim

    Exotic atomic nuclei far away from stability are fascinating objects to be studied in many scientic elds such as atomic-, nuclear-, and astrophysics. Since these are often short-lived isotopes, it is necessary to couple their production with immediate extraction and delivery to an experiment. This is the purpose of the on-line isotope separator facility, ISOLDE, at CERN. An essential aspect of this laboratory is the Resonance Ionization Laser Ion Source (RILIS) because it provides a fast and highly selective means of ionizing the reaction products. This technique is also a sensitive laser-spectroscopy tool for the development and improvement of electron excitation schemes for the resonant laser photoionization and the study of the nuclear structure or fundamental atomic physics. Each of these aspects of the RILIS applications are subjects of this thesis work: a new device for the suppression of unwanted surface ionized contaminants in RILIS ion beams, known as the Laser Ion Source and Trap (LIST), was impleme...

  2. A homogeneous assay for highly sensitive detection of CaMV35S promoter in transgenic soybean by förster resonance energy transfer between nitrogen-doped graphene quantum dots and Ag nanoparticles.

    Science.gov (United States)

    Li, Yaqi; Sun, Li; Qian, Jing; Wang, Chengke; Liu, Qian; Han, En; Hao, Nan; Zhang, Liuping; Cai, Jianrong; Wang, Kun

    2016-12-15

    In this work, a novel homogeneous assay for DNA quantitative analysis based on förster resonance energy transfer (FRET) was developed for cauliflwer mosaic virus 35s (CaMV35S) promoter of transgenic soybean detection. The homogenous FRET of fluorescence signal was fabricated by DNA hybridization with probe modified nitrogen-doped graphene quantum dots (NGQDs) and silver nanoparticles (AgNPs), which acted the donor-acceptor pairs for the first time. The highly efficient FRET and unique properties of the NGQDs made the proposed FRET system as a functionalized detection platform for labelling of DNA. Upon the recognition of specific target DNA (tDNA), the FRET between NGQDs and AgNPs was triggered to produce fluorescence quenching, which could be used for tDNA detection. The fabricated homogeneous FRET assay displayed a wide linear range of 0.1-500.0 nM and a low limit of detection 0.03 nM for the detection of CaMV35S (S/N = 3). This proposed biosensor revealed high specificity to detect tDNA, with acceptable intra-assay precision and excellent stability. This method was successfully applied to identify the real sample of 0.5% containing transgenic soybean, which achieved the most of national law regulations. This assay was further validated by polymerase chain reaction as the genetically modified organisms, suggesting that the proposed FRET system is a feasible tool for the further daily genetically modified organism detection. Copyright © 2016 Elsevier B.V. All rights reserved.

  3. Time differentiated nuclear resonance spectroscopy coupled with pulsed laser heating in diamond anvil cells

    Energy Technology Data Exchange (ETDEWEB)

    Kupenko, I., E-mail: kupenko@esrf.fr; Strohm, C. [Bayerisches Geoinstitut, Universität Bayreuth, D-95440 Bayreuth (Germany); ESRF-The European Synchrotron, CS 40220, 38043 Grenoble Cedex 9 (France); McCammon, C.; Cerantola, V.; Petitgirard, S.; Dubrovinsky, L. [Bayerisches Geoinstitut, Universität Bayreuth, D-95440 Bayreuth (Germany); Glazyrin, K. [Photon Science, DESY, D-22607 Hamburg (Germany); Vasiukov, D.; Aprilis, G. [Laboratory of Crystallography, Material Physics and Technology at Extreme Conditions, Universität Bayreuth, D-95440 Bayreuth (Germany); Chumakov, A. I.; Rüffer, R. [ESRF-The European Synchrotron, CS 40220, 38043 Grenoble Cedex 9 (France)

    2015-11-15

    Developments in pulsed laser heating applied to nuclear resonance techniques are presented together with their applications to studies of geophysically relevant materials. Continuous laser heating in diamond anvil cells is a widely used method to generate extreme temperatures at static high pressure conditions in order to study the structure and properties of materials found in deep planetary interiors. The pulsed laser heating technique has advantages over continuous heating, including prevention of the spreading of heated sample and/or the pressure medium and, thus, a better stability of the heating process. Time differentiated data acquisition coupled with pulsed laser heating in diamond anvil cells was successfully tested at the Nuclear Resonance beamline (ID18) of the European Synchrotron Radiation Facility. We show examples applying the method to investigation of an assemblage containing ε-Fe, FeO, and Fe{sub 3}C using synchrotron Mössbauer source spectroscopy, FeCO{sub 3} using nuclear inelastic scattering, and Fe{sub 2}O{sub 3} using nuclear forward scattering. These examples demonstrate the applicability of pulsed laser heating in diamond anvil cells to spectroscopic techniques with long data acquisition times, because it enables stable pulsed heating with data collection at specific time intervals that are synchronized with laser pulses.

  4. Laser mit instabilem Resonator fuer ringfoermige aktive Medien

    OpenAIRE

    Jarosch, U.K.; Habich, U.; Plum, H.D.

    1996-01-01

    Beschrieben werden Laser mit instabilen Resonatoren, die ringfoermige Medien effektiv ausnutzen, unabhaengig davon, ob es sich um feste, fluessige oder gasfoermige Medien handelt. Die Erfindung zeichnet sich dadurch aus, dass die Auskopplung des Strahles (5.1) eines Ringresonators entlang eines Spaltes oder eines Kreisringes ueber dem gesamten Umfang vorgesehen ist, wobei der Laserresonator durch Ringspiegel (1,2) mit torusfoermiger Spiegelflaeche gebildet und von den Waenden des Ringspaltes ...

  5. Resonantly-pumped soft-x-ray lasers using ICF drivers

    International Nuclear Information System (INIS)

    Hagelstein, P.L.

    1982-12-01

    Some aspects of laser design relating to experiments planned for the NOVETTE laser system at Livermore in early 1983 are discussed. The experiments are aimed at testing several resonantly-pumped lasers with transition energies between 42.3 eV and 153 eV. These experiments follow several years of theoretical work, a set of flashlamp characterization experiments performed on the SHIVA laser system (LLNL) in December, 1981, and some high precision spectroscopic studies carried out at KMS during the summer of 1982. Some of the major physics design issues as the relate to the experiments, and some of the numerical simulations that have been carried out so far are reviewed

  6. On formation of a partially coherent beam in a stable-resonator laser

    International Nuclear Information System (INIS)

    Suvorov, A A

    2010-01-01

    A new method involving the expansion of the field coherence function in partially coherent modes - the eigensolutions of the problem for the second-order coherence function in a stable resonator - is proposed for the theoretical description of the process of multimode laser beam formation. The method for solving the problem for arbitrary partially coherent modes is formulated and the expressions for these modes are derived in the general form. The characteristics of the fundamental partially coherent mode, which coincides with the coherence function of a Gaussian partially coherent beam, are analysed in detail. The partially coherent modes are shown to possess two spatial scales - the effective radius and the coherence radius, which makes them a convenient tool for solving the problem of generation of a partially coherent beam. It is found that the unambiguous relation between the characteristics of partially coherent modes and the stable-resonator parameters is achieved by involving into consideration not only the process of the beam formation by the resonator mirrors but also the process of interaction of radiation with the active laser medium. (laser beams and resonators)

  7. Spectroscopic investigations of novel pharmaceuticals: Stability and resonant interaction with laser beam

    Science.gov (United States)

    Smarandache, Adriana; Boni, Mihai; Andrei, Ionut Relu; Handzlik, Jadwiga; Kiec-Kononowicz, Katarzyna; Staicu, Angela; Pascu, Mihail-Lucian

    2017-09-01

    This paper presents data about photophysics of two novel thio-hydantoins that exhibit promising pharmaceutical properties in multidrug resistance control. Time stability studies are necessary to establish the proper use of these compounds in different applications. As for their administration as drugs, it is imperative to know their shelf life, as well as storage conditions. At the same time, laser induced modified properties of the two new compounds are valuable to further investigate their specific interactions with other materials, including biological targets. The two new thio-hydantoins under generic names SZ-2 and SZ-7 were prepared as solutions in dimethyl sulfoxide at different concentrations, as well as in deionised water. For the stability assay they were kept in various light/temperature conditions up to 60 days. The stability was estimates based on UV-vis absorption measurements. The samples in bulk shape were exposed different time intervals to laser radiation emitted at 266 nm as the fourth harmonic of a Nd:YAG laser. The resonant interaction of the studied compounds with laser beams was analysed through spectroscopic methods UV-vis and FTIR absorption, as well as laser induced fluorescence spectroscopy. As for stability assay, only solutions kept in dark at 4 °C have preserved the absorption characteristics, considering the cumulated measuring errors, less than one week. The vibrational changes that occur in their FTIR and modified fluorescence spectra upon laser beam exposure are also discussed. A result of the experimental analysis is that modifications are induced in molecular structures of the investigated compounds by resonant interaction with laser radiation. This fact evidences that the molecules are photoreactive and their characteristics might be shaped through controlled laser radiation exposure using appropriate protocols. This conclusion opens many opportunities both in the biomedical field, but also in other industrial activities

  8. Self-resonant wakefield excitation by intense laser pulse in plasmas

    International Nuclear Information System (INIS)

    Andreev, N.E.; Pogosova, A.A.; Gorbunov, L.M.; Ramazashvili, R.R.; Kirsanov, V.I.

    1993-01-01

    It is demonstrated by theoretical analysis and numerical calculations that in an underdense plasma the process of three-dimensional evolution of the short and strong laser pulse (with duration equal to several plasma periods) leads to compression and self-modulation of the pulse, so that during a fairly long period of time beats of pulse amplitude generates resonantly a strong and stable plasma wakefield. The intensity of the wake-field is so high that it can provide a new promising outlook for the plasma based accelerator concept. Linear analysis of dispersion relation predicts that taking into account transverse component of wavenumber considerably increases the growth rate of resonance instability of the pulse. The numerical simulations demonstrate that considered self-focusing and resonant-modulation instability are essentially three dimensional processes. Laser field evolution in each transverse cross section of the pulse is synchronized by the regular structure of plasma wave that is excited by the pulse. The considered effect of resonant modulation has a threshold. For the pulses with the intensity below the threshold the refraction dominates and no modulation appears. The studied phenomenon can be referred to as the Self-Resonant Wakefield (SRWF) excitation that is driven by self-focusing and self-modulation of laser pulse with quite a moderate initial duration. In fact, this method of excitation differs from both suggested in Ref.1 (PBWA) and in Refs.2,3 (LWFA), being even more than the combination of these concepts. Unlike the first scheme it does not require initially the two-frequency laser pulse, since the modulation here appears in the most natural way due to evolution of the pulse. In contrast with the LWFA, the considered SRWF generation scheme gives the possibility to raise the intensity of wake-excitation due to pulse self-focusing ( initial stage) and self modulation (second stage)

  9. Laser heating of large noble gas clusters: from the resonant to the relativistic interaction regimes

    Energy Technology Data Exchange (ETDEWEB)

    Gumbrell, E T; Moore, A S; Clark, E L; Garbett, W J; Comley, A J; Edwards, R D; Eagleton, R E [Plasma Physics Division, AWE Aldermaston, Reading RG7 4PR (United Kingdom); Lazarus, J A; Nilson, P M; Robinson, J S; Hohenberger, M; Symes, D R; Smith, R A [Blackett Laboratory, Imperial College, London SW7 2BZ (United Kingdom); Clarke, R J [Rutherford Appleton Laboratory, Chilton OX11 0QX (United Kingdom)], E-mail: edward.gumbrell@awe.co.uk, E-mail: r.a.smith@imperial.ac.uk

    2008-12-15

    Wide-ranging measurements of sub-picosecond laser interactions with large noble gas cluster targets have been conducted in order to help clarify the nature and extent of the underlying laser-plasma heating. Within the sub-relativistic vacuum irradiance range of 10{sup 16}-10{sup 17} W cm{sup -2}, we find that electron temperatures measured with continuum x-ray spectroscopy exhibit a pronounced multi-keV enhancement. Analysis indicates this behaviour to be consistent with collisional or collisionless resonant heating mechanisms. We also present the first measurements of laser-to-cluster energy deposition at relativistic vacuum irradiances, our data demonstrating absorption fractions of 90% or more. Optical probing was used to resolve the onset of a supersonic ionization front resulting from this very high absorption, and shows that despite significant pre-focus heating, the greatest plasma energy densities can be generated about the vacuum focus position. Electron energy spectra measurements confirm that laser-plasma super-heating occurs, and together with ion data establish that relativistic laser-plasma coupling in atomic clusters can take place without significant MeV particle beam production. In conjunction with optical self-emission data, the optical probing also indicates laser pre-pulse effects at peak vacuum irradiance of 5 x 10{sup 19} W cm{sup -2}. Laser absorption, plasma heating and energy transport data are supported throughout with analytical and numerical modelling.

  10. Study on VCSEL laser heating chip in nuclear magnetic resonance gyroscope

    Science.gov (United States)

    Liang, Xiaoyang; Zhou, Binquan; Wu, Wenfeng; Jia, Yuchen; Wang, Jing

    2017-10-01

    In recent years, atomic gyroscope has become an important direction of inertial navigation. Nuclear magnetic resonance gyroscope has a stronger advantage in the miniaturization of the size. In atomic gyroscope, the lasers are indispensable devices which has an important effect on the improvement of the gyroscope performance. The frequency stability of the VCSEL lasers requires high precision control of temperature. However, the heating current of the laser will definitely bring in the magnetic field, and the sensitive device, alkali vapor cell, is very sensitive to the magnetic field, so that the metal pattern of the heating chip should be designed ingeniously to eliminate the magnetic field introduced by the heating current. In this paper, a heating chip was fabricated by MEMS process, i.e. depositing platinum on semiconductor substrates. Platinum has long been considered as a good resistance material used for measuring temperature The VCSEL laser chip is fixed in the center of the heating chip. The thermometer resistor measures the temperature of the heating chip, which can be considered as the same temperature of the VCSEL laser chip, by turning the temperature signal into voltage signal. The FPGA chip is used as a micro controller, and combined with PID control algorithm constitute a closed loop control circuit. The voltage applied to the heating resistor wire is modified to achieve the temperature control of the VCSEL laser. In this way, the laser frequency can be controlled stably and easily. Ultimately, the temperature stability can be achieved better than 100mK.

  11. Resonant ablation of single-wall carbon nanotubes by femtosecond laser pulses

    International Nuclear Information System (INIS)

    Arutyunyan, N R; Komlenok, M S; Kononenko, V V; Pashinin, V P; Pozharov, A S; Konov, V I; Obraztsova, E D

    2015-01-01

    The thin 50 nm film of bundled arc-discharge single-wall carbon nanotubes was irradiated by femtosecond laser pulses with wavelengths 675, 1350 and 1745 nm corresponding to the absorption band of metallic nanotubes E 11 M , to the background absorption and to the absorption band of semiconducting nanotubes E 11 S , respectively. The aim was to induce a selective removal of nanotubes of specific type from the bundled material. Similar to conducted thermal heating experiments, the effect of laser irradiation results in suppression of all radial breathing modes in the Raman spectra, with preferential destruction of the metallic nanotubes with diameters less than 1.26 nm and of the semiconducting nanotubes with diameters 1.36 nm. However, the etching rate of different nanotubes depends on the wavelength of the laser irradiation. It is demonstrated that the relative content of nanotubes of different chiralities can be tuned by a resonant laser ablation of undesired nanotube fraction. The preferential etching of the resonant nanotubes has been shown for laser wavelengths 675 nm (E 11 M ) and 1745 nm (E 11 S ). (paper)

  12. Modeling of mode-locked coupled-resonator optical waveguide lasers

    DEFF Research Database (Denmark)

    Agger, Christian; Skovgård, Troels Suhr; Gregersen, Niels

    2010-01-01

    Coupled-resonator optical waveguides made from coupled high-Q photonic crystal nanocavities are investigated for use as cavities in mode-locked lasers. Such devices show great potential in slowing down light and can serve to reduce the cavity length of a mode-locked laser. An explicit expression...... of the emerging pulse train. A range of tuning around this frequency allows for effective mode locking. Finally, noise is added to the generalized single-cavity eigenfrequencies in order to evaluate the effects of fabrication imperfections on the cold-cavity transmission properties and consequently on the locking...

  13. Wavelength-controlled external-cavity laser with a silicon photonic crystal resonant reflector

    Science.gov (United States)

    Gonzalez-Fernandez, A. A.; Liles, Alexandros A.; Persheyev, Saydulla; Debnath, Kapil; O'Faolain, Liam

    2016-03-01

    We report the experimental demonstration of an alternative design of external-cavity hybrid lasers consisting of a III-V Semiconductor Optical Amplifier with fiber reflector and a Photonic Crystal (PhC) based resonant reflector on SOI. The Silicon reflector comprises a polymer (SU8) bus waveguide vertically coupled to a PhC cavity and provides a wavelength-selective optical feedback to the laser cavity. This device exhibits milliwatt-level output power and sidemode suppression ratio of more than 25 dB.

  14. Laser resonance ionization scheme development for tellurium and germanium at the dual Ti:Sa–Dye ISOLDE RILIS

    Energy Technology Data Exchange (ETDEWEB)

    Day Goodacre, T., E-mail: thomas.day.goodacre@cern.ch [CERN, CH-1211 Geneva 23 (Switzerland); School of Physics and Astronomy, The University of Manchester, Manchester M13 9PL (United Kingdom); Fedorov, D. [Petersburg Nuclear Physics Institute, 188350 Gatchina (Russian Federation); Fedosseev, V.N.; Forster, L.; Marsh, B.A. [CERN, CH-1211 Geneva 23 (Switzerland); Rossel, R.E. [CERN, CH-1211 Geneva 23 (Switzerland); Institut für Physik, Johannes Gutenberg Universität, D-55099 Mainz (Germany); Faculty of Design, Computer Science and Media, Hochschule RheinMain, Wiesbaden (Germany); Rothe, S.; Veinhard, M. [CERN, CH-1211 Geneva 23 (Switzerland)

    2016-09-11

    The resonance ionization laser ion source (RILIS) is the principal ion source of the ISOLDE radioactive beam facility based at CERN. Using the method of in-source laser resonance ionization spectroscopy, a transition to a new autoionizing state of tellurium was discovered and applied as part of a three-step, three-resonance, photo-ionization scheme. In a second study, a three-step, two-resonance, photo-ionization scheme for germanium was developed and the ionization efficiency was measured at ISOLDE. This work increases the range of ISOLDE RILIS ionized beams to 31 elements. Details of the spectroscopy studies are described and the new ionization schemes are summarized.

  15. Laser resonance ionization scheme development for tellurium and germanium at the dual Ti:Sa–Dye ISOLDE RILIS

    CERN Document Server

    Day Goodacre, T.; Fedosseev, V.N.; Forster, L.; Marsh, B.A.; Rossel, R.E.; Rothe, S.; Veinhard, M.

    2016-01-01

    The resonance ionization laser ion source (RILIS) is the principal ion source of the ISOLDE radioactive beam facility based at CERN. Using the method of in-source laser resonance ionization spectroscopy, a transition to a new autoionizing state of tellurium was discovered and applied as part of a three-step, three-resonance, photo-ionization scheme. In a second study, a three-step, two-resonance, photo-ionization scheme for germanium was developed and the ionization efficiency was measured at ISOLDE. This work increases the range of ISOLDE RILIS ionized beams to 31 elements. Details of the spectroscopy studies are described and the new ionization schemes are summarized.

  16. Lasers

    CERN Document Server

    Milonni, Peter W

    1988-01-01

    A comprehensive introduction to the operating principles and applications of lasers. Explains basic principles, including the necessary elements of classical and quantum physics. Provides concise discussions of various laser types including gas, solid state, semiconductor, and free electron lasers, as well as of laser resonators, diffraction, optical coherence, and many applications including holography, phase conjugation, wave mixing, and nonlinear optics. Incorporates many intuitive explanations and practical examples. Discussions are self-contained in a consistent notation and in a style that should appeal to physicists, chemists, optical scientists and engineers.

  17. Resonant-enhanced above-threshold ionization of atoms by XUV short laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Rodriguez, V.D. [Departamento de Fisica, FCEyN, Universidad de Buenos Aires, 1428 Buenos Aires (Argentina)], E-mail: vladimir@df.uba.ar; Macri, P.A. [Instituto de Investigaciones Fisicas de Mar del Plata (IFIMAR), Departamento de Fisica, FCEyN, Universidad Nacional de Mar del Plata, CONICET, Funes 3350, 7600 Mar del Plata (Argentina); Arbo, D.G. [Instituto de Astronomia y Fisica del Espacio, UBA-CONICET, CC 67 Suc 28 Buenos Aires (Argentina)

    2009-01-15

    Above-threshold ionization of atoms by XUV short laser pulses is investigated close to the resonant 1s-2p transitions. Both ab initio TDSE and a theoretical Coulomb-Volkov like theory are used to study the enhancement in the ionization probabilities. Our modified Coulomb-Volkov theory, fully accounting for the important 1s-2p transition is able to explain the spectrum as well as the total ionization cross sections.

  18. Proton emission from resonant laser absorption and self-focusing effects from hydrogenated structures

    Czech Academy of Sciences Publication Activity Database

    Cutroneo, M.; Torrisi, L.; Margarone, Daniele; Picciotto, A.

    2013-01-01

    Roč. 272, May (2013), s. 50-54 ISSN 0169-4332 R&D Projects: GA MŠk EE.2.3.20.0087 Grant - others:OP VK 2 LaserGen(XE) CZ.1.07/2.3.00/20.0087 Institutional support: RVO:68378271 Keywords : resonant absorption * self-focusing * Thomson parabola * spectrometer Subject RIV: BL - Plasma and Gas Discharge Physics Impact factor: 2.538, year: 2013

  19. Experimental investigations of driven Alfven wave resonances in a tokamak plasma using carbon dioxide laser interferometry

    International Nuclear Information System (INIS)

    Evans, T.E.

    1984-09-01

    The first direct observation of the internal structure of driven global Alfven eigenmodes in a tokamak plasma is presented. A carbon dioxide laser scattering/interferometer has been designed, built, and installed on the PRETEXT tokamak. By using this diagnostic system in the interferometer configuration, we have for the first time, thoroughly investigated the resonance conditions required for, and the spatial wave field structure of, driven plasma eigenmodes at frequencies below the ion cyclotron frequency in a confined, high temperature, tokamak plasma

  20. Collinear resonant ionization laser spectroscopy of rare francium isotopes

    CERN Multimedia

    Neyens, G; Flanagan, K; Rajabali, M M; Le blanc, F M; Ware, T; Procter, T J

    2008-01-01

    We propose a programme of collinear resonant ionization spectroscopy (CRIS) of the francium isotopes up to and including $^{201}$Fr and $^{218,219}$Fr. This work aims at answering questions on the ordering of quantum states, and effect of the ($\\pi s_{1/2}^{-1}$)1/2$^{+}$ intruder state, which is currently believed to be the ground state of $^{199}$Fr. This work will also study the edge of the region of reflection asymmetry through measurement of the moments and radii of $^{218,219}$Fr. This proposal forms the first part of a series of experiments that will study nuclei in this region of the nuclear chart. Based on the success of this initial proposal it is the intention of the collaboration to perform high resolution measurements on the isotopes of radium and radon that surround $^{201}$Fr and $^{218}$Fr and thus providing a comprehensive description of the ground state properties of this region of the nuclear chart. Recent in-source spectroscopy measurements of lead, bismuth and polonium have demonstrated a...

  1. Heterogeneous catalysis in highly sensitive microreactors

    DEFF Research Database (Denmark)

    Olsen, Jakob Lind

    This thesis present a highly sensitive silicon microreactor and examples of its use in studying catalysis. The experimental setup built for gas handling and temperature control for the microreactor is described. The implementation of LabVIEW interfacing for all the experimental parts makes...

  2. Aluminum nanocantilevers for high sensitivity mass sensors

    DEFF Research Database (Denmark)

    Davis, Zachary James; Boisen, Anja

    2005-01-01

    We have fabricated Al nanocantilevers using a simple, one mask contact UV lithography technique with lateral and vertical dimensions under 500 and 100 nm, respectively. These devices are demonstrated as highly sensitive mass sensors by measuring their dynamic properties. Furthermore, it is shown ...

  3. Efficient 525 nm laser generation in single or double resonant cavity

    Science.gov (United States)

    Liu, Shilong; Han, Zhenhai; Liu, Shikai; Li, Yinhai; Zhou, Zhiyuan; Shi, Baosen

    2018-03-01

    This paper reports the results of a study into highly efficient sum frequency generation from 792 and 1556 nm wavelength light to 525 nm wavelength light using either a single or double resonant ring cavity based on a periodically poled potassium titanyl phosphate crystal (PPKTP). By optimizing the cavity's parameters, the maximum power achieved for the resultant 525 nm laser was 263 and 373 mW for the single and double resonant cavity, respectively. The corresponding quantum conversion efficiencies were 8 and 77% for converting 1556 nm photons to 525 nm photons with the single and double resonant cavity, respectively. The measured intra-cavity single pass conversion efficiency for both configurations was about 5%. The performances of the sum frequency generation in these two configurations was studied and compared in detail. This work will provide guidelines for optimizing the generation of sum frequency generated laser light for a variety of configurations. The high conversion efficiency achieved in this work will help pave the way for frequency up-conversion of non-classical quantum states, such as the squeezed vacuum and single photon states. The proposed green laser source will be used in our future experiments, which includes a plan to generate two-color entangled photon pairs and achieve the frequency down-conversion of single photons carrying orbital angular momentum.

  4. Wafer-level vacuum packaged resonant micro-scanning mirrors for compact laser projection displays

    Science.gov (United States)

    Hofmann, Ulrich; Oldsen, Marten; Quenzer, Hans-Joachim; Janes, Joachim; Heller, Martin; Weiss, Manfred; Fakas, Georgios; Ratzmann, Lars; Marchetti, Eleonora; D'Ascoli, Francesco; Melani, Massimiliano; Bacciarelli, Luca; Volpi, Emilio; Battini, Francesco; Mostardini, Luca; Sechi, Francesco; De Marinis, Marco; Wagner, Bernd

    2008-02-01

    Scanning laser projection using resonant actuated MEMS scanning mirrors is expected to overcome the current limitation of small display size of mobile devices like cell phones, digital cameras and PDAs. Recent progress in the development of compact modulated RGB laser sources enables to set up very small laser projection systems that become attractive not only for consumer products but also for automotive applications like head-up and dash-board displays. Within the last years continuous progress was made in increasing MEMS scanner performance. However, only little is reported on how mass-produceability of these devices and stable functionality even under harsh environmental conditions can be guaranteed. Automotive application requires stable MEMS scanner operation over a wide temperature range from -40° to +85°Celsius. Therefore, hermetic packaging of electrostatically actuated MEMS scanning mirrors becomes essential to protect the sensitive device against particle contamination and condensing moisture. This paper reports on design, fabrication and test of a resonant actuated two-dimensional micro scanning mirror that is hermetically sealed on wafer level. With resonant frequencies of 30kHz and 1kHz, an achievable Theta-D-product of 13mm.deg and low dynamic deformation <20nm RMS it targets Lissajous projection with SVGA-resolution. Inevitable reflexes at the vacuum package surface can be seperated from the projection field by permanent inclination of the micromirror.

  5. Selective isotope determination of lanthanum by diode-laser-initiated resonance-ionization mass spectrometry

    International Nuclear Information System (INIS)

    Young, J.P.; Shaw, R.W.

    1995-01-01

    A diode-laser step has been incorporated into a resonance-ionization mass spectrometry optical excitation process to enhance the isotopic selectivity of the technique. Lanthanum isotope ratio enhancements as high as 10 3 were achieved by use of a single-frequency cw diode laser tuned to excite the first step of a three-step excitation--ionization optical process; the subsequent steps were excited by use of a pulsed dye laser. Applying the same optical technique, we measured atomic hyperfine constants for the high-lying even-parity 4 D 5/2 state of lanthanum at 30 354 cm --1 . The general utility of this spectral approach is discussed

  6. Parallel ion flow velocity measurement using laser induced fluorescence method in an electron cyclotron resonance plasma

    International Nuclear Information System (INIS)

    Yoshimura, Shinji; Okamoto, Atsushi; Terasaka, Kenichiro; Ogiwara, Kohei; Tanaka, Masayoshi Y.; Aramaki, Mitsutoshi

    2010-01-01

    Parallel ion flow velocity along a magnetic field has been measured using a laser induced fluorescence (LIF) method in an electron cyclotron resonance (ECR) argon plasma with a weakly-diverging magnetic field. To measure parallel flow velocity in a cylindrical plasma using the LIF method, the laser beam should be injected along device axis; however, the reflection of the incident beam causes interference between the LIF emission of the incident and reflected beams. Here we present a method of quasi-parallel laser injection at a small angle, which utilizes the reflected beam as well as the incident beam to obtain the parallel ion flow velocity. Using this method, we observed an increase in parallel ion flow velocity along the magnetic field. The acceleration mechanism is briefly discussed on the basis of the ion fluid model. (author)

  7. Resonant third-harmonic generation of a short-pulse laser from electron-hole plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Kant, Niti [Department of Physics, Lovely Professional University, Phagwara, Punjab 144 402 (India); Nandan Gupta, Devki [Department of Physics and Astrophysics, University of Delhi, Delhi 110 007 (India); Suk, Hyyong [Advanced Photonics Research Institute (APRI) and Graduate Program of Photonics and Applied Physics, Gwangju Institute of Science and Technology, Gwangju 500 712 (Korea, Republic of)

    2012-01-15

    In semiconductors, free carriers are created in pairs in inter-band transitions and consist of an electron and its corresponding hole. At very high carrier densities, carrier-carrier collisions dominate over carrier-lattice collisions and carriers begin to behave collectively to form plasma. Here, we apply a short-pulse laser to generate third-harmonic radiation from a semiconductor plasma (electron-hole plasma) in the presence of a transverse wiggler magnetic-field. The process of third-harmonic generation of an intense short-pulse laser is resonantly enhanced by the magnetic wiggler, i.e., wiggler magnetic field provides the necessary momentum to third-harmonic photons. In addition, a high-power laser radiation, propagating through a semiconductor imparts an oscillatory velocity to the electrons and exerts a ponderomotive force on electrons at the third-harmonic frequency of the laser. This oscillatory velocity produces a third-harmonic longitudinal current. And due to the beating of the longitudinal electron velocity and the wiggler magnetic field, a transverse third-harmonic current is produced that drives third-harmonic electromagnetic radiation. It is finally observed that for a specific wiggler wave number value, the phase-matching conditions for the process are satisfied, leading to resonant enhancement in the energy conversion efficiency.

  8. Resonant third-harmonic generation of a short-pulse laser from electron-hole plasmas

    International Nuclear Information System (INIS)

    Kant, Niti; Nandan Gupta, Devki; Suk, Hyyong

    2012-01-01

    In semiconductors, free carriers are created in pairs in inter-band transitions and consist of an electron and its corresponding hole. At very high carrier densities, carrier-carrier collisions dominate over carrier-lattice collisions and carriers begin to behave collectively to form plasma. Here, we apply a short-pulse laser to generate third-harmonic radiation from a semiconductor plasma (electron-hole plasma) in the presence of a transverse wiggler magnetic-field. The process of third-harmonic generation of an intense short-pulse laser is resonantly enhanced by the magnetic wiggler, i.e., wiggler magnetic field provides the necessary momentum to third-harmonic photons. In addition, a high-power laser radiation, propagating through a semiconductor imparts an oscillatory velocity to the electrons and exerts a ponderomotive force on electrons at the third-harmonic frequency of the laser. This oscillatory velocity produces a third-harmonic longitudinal current. And due to the beating of the longitudinal electron velocity and the wiggler magnetic field, a transverse third-harmonic current is produced that drives third-harmonic electromagnetic radiation. It is finally observed that for a specific wiggler wave number value, the phase-matching conditions for the process are satisfied, leading to resonant enhancement in the energy conversion efficiency.

  9. Enhancement of optical Kerr effect in quantum-cascade lasers with multiple resonance levels.

    Science.gov (United States)

    Bai, Jing; Citrin, D S

    2008-08-18

    In this paper, we investigated the optical Kerr lensing effect in quantum-cascade lasers with multiple resonance levels. The Kerr refractive index n2 is obtained through the third-order susceptibility at the fundamental frequency chi(3)( omega; omega, omega,-omega). Resonant two-photon processes are found to have almost equal contributions to chi(3)( omega; omega, omega,-omega) as the single-photon processes, which result in the predicted enhancement of the positive nonlinear (Kerr) refractive index, and thus may enhance mode-locking of quantum-cascade lasers. Moreover, we also demonstrate an isospectral optimization strategy for further improving n2 through the band-structure design, in order to boost the multimode performance of quantum-cascade lasers. Simulation results show that the optimized stepwise multiple-quantum-well structure has n2 approximately 10-8 cm2/W, a twofold enhancement over the original flat quantum-well structure. This leads to a refractive-index change (delta)n of about 0.01, which is at the upper bound of those reported for typical Kerr medium. This stronger Kerr refractive index may be important for quantum-cascade lasers ultimately to demonstrate self-mode-locking.

  10. Evaluation of thermal effects on the beam quality of disk laser with unstable resonator

    Science.gov (United States)

    Shayganmanesh, Mahdi; Beirami, Reza

    2017-01-01

    In this paper thermal effects of the disk active medium and associated effects on the beam quality of laser are investigated. Using Collins integral and iterative method, transverse mode of an unstable resonator including a Yb:YAG active medium in disk geometry is calculated. After that the beam quality of the laser is calculated based on the generalized beam characterization method. Thermal lensing of the disk is calculated based on the OPD (Optical Path Difference) concept. Five factors influencing the OPD including temperature gradient, disk thermal expansion, photo-elastic effect, electronic lens and disk deformation are considered in our calculations. The calculations show that the effect of disk deformation factor on the quality of laser beam in the resonator is strong. However the total effect of all the thermal factors on the internal beam quality is fewer. Also it is shown that thermal effects degrade the output power, beam profile and beam quality of the output laser beam severely. As well the magnitude of each of affecting factors is evaluated distinctly.

  11. In situ sulfur isotopes (δ{sup 34}S and δ{sup 33}S) analyses in sulfides and elemental sulfur using high sensitivity cones combined with the addition of nitrogen by laser ablation MC-ICP-MS

    Energy Technology Data Exchange (ETDEWEB)

    Fu, Jiali [State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Wuhan 430074 (China); Hu, Zhaochu, E-mail: zchu@vip.sina.com [State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Wuhan 430074 (China); The Beijing SHRIMP Center, Institute of Geology, Chinese Academy of Geological Sciences, Beijing 102206 (China); Zhang, Wen [State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Wuhan 430074 (China); Yang, Lu [State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Wuhan 430074 (China); National Research Council Canada, 1200 Montreal Rd., Ottawa, Ontario K1A 0R6 (Canada); Liu, Yongsheng; Li, Ming; Zong, Keqing; Gao, Shan; Hu, Shenghong [State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Wuhan 430074 (China)

    2016-03-10

    The sulfur isotope is an important geochemical tracer in diverse fields of geosciences. In this study, the effects of three different cone combinations with the addition of N{sub 2} on the performance of in situ S isotope analyses were investigated in detail. The signal intensities of S isotopes were improved by a factor of 2.3 and 3.6 using the X skimmer cone combined with the standard sample cone or the Jet sample cone, respectively, compared with the standard arrangement (H skimmer cone combined with the standard sample cone). This signal enhancement is important for the improvement of the precision and accuracy of in situ S isotope analysis at high spatial resolution. Different cone combinations have a significant effect on the mass bias and mass bias stability for S isotopes. Poor precisions of S isotope ratios were obtained using the Jet and X cones combination at their corresponding optimum makeup gas flow when using Ar plasma only. The addition of 4–8 ml min{sup −1} nitrogen to the central gas flow in laser ablation MC-ICP-MS was found to significantly enlarge the mass bias stability zone at their corresponding optimum makeup gas flow in these three different cone combinations. The polyatomic interferences of OO, SH, OOH were also significantly reduced, and the interference free plateaus of sulfur isotopes became broader and flatter in the nitrogen mode (N{sub 2} = 4 ml min{sup −1}). However, the signal intensity of S was not increased by the addition of nitrogen in this study. The laser fluence and ablation mode had significant effects on sulfur isotope fractionation during the analysis of sulfides and elemental sulfur by laser ablation MC-ICP-MS. The matrix effect among different sulfides and elemental sulfur was observed, but could be significantly reduced by line scan ablation in preference to single spot ablation under the optimized fluence. It is recommended that the d{sub 90} values of the particles in pressed powder pellets for accurate

  12. Investigation of natural frequencies of laser inertial confinement fusion capsules using resonant ultrasound spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Ma, Xiaojun [Institute of Modern Physics, Fudan University, Shanghai 200433 (China); Research Center of Laser Fusion, CAEP, Mianyang 621900 (China); Tang, Xing; Wang, Zongwei [Research Center of Laser Fusion, CAEP, Mianyang 621900 (China); Chen, Qian; Qian, Menglu [Institute of Acoustic, Tongji University, Shanghai 200433 (China); Meng, Jie [Research Center of Laser Fusion, CAEP, Mianyang 621900 (China); Tang, Yongjian [Institute of Modern Physics, Fudan University, Shanghai 200433 (China); Research Center of Laser Fusion, CAEP, Mianyang 621900 (China); Zou, Yaming; Shen, Hao [Institute of Modern Physics, Fudan University, Shanghai 200433 (China); Gao, Dangzhong, E-mail: dgaocn@163.com [Research Center of Laser Fusion, CAEP, Mianyang 621900 (China)

    2017-01-15

    Highlights: • The frequency equation of isotropic multi-layer hollow spheres was derived using three-dimension (3D) elasticity theory and transfer matrix method. • The natural frequencies of the capsules with a millimeter-sized diameter are determined experimentally using resonant ultrasound spectrum (RUS) system. • The predicted natural frequencies of the frequency equation accord well with the observed results. • The theoretical and experimental investigation has proved the potential applicability of RUS to both metallic and non-metallic capsules. - Abstract: The natural frequency problem of laser inertial confinement fusion (ICF) capsules is one of the basic problems for determining non-destructively the elasticity modulus of each layer material using resonant ultrasound spectroscopy (RUS). In this paper, the frequency equation of isotropic one-layer hollow spheres was derived using three dimension (3D) elasticity theory and some simplified frequency equations were discussed under axisymmetric and spherical symmetry conditions. The corresponding equation of isotropic multi-layer hollow spheres was given employing transfer matrix method. To confirm the validity of the frequency equation and explore the feasibility of RUS for characterizing the ICF capsules, three representative capsules with a millimeter-sized diameter were determined by piezoelectric-based resonant ultrasound spectroscopy (PZT-RUS) and laser-based resonant ultrasound spectroscopy (LRUS) techniques. On the basis of both theoretical and experimental results, it is proved that the calculated and measured natural frequencies are accurate enough for determining the ICF capsules.

  13. Nuclear magnetic resonance of laser-polarized noble gases in molecules, materials and organisms

    International Nuclear Information System (INIS)

    Goodson, Boyd M.

    1999-01-01

    Conventional nuclear magnetic resonance (NMR) spectroscopy and magnetic resonance imaging (MRI) are fundamentally challenged by the insensitivity that stems from the ordinarily low spin polarization achievable in even the strongest NMR magnets. However, by transferring angular momentum from laser light to electronic and nuclear spins, optical pumping methods can increase the nuclear spin polarization of noble gases by several orders of magnitude, thereby greatly enhancing their NMR sensitivity. This dissertation is primarily concerned with the principles and practice of optically pumped nuclear magnetic resonance (OPNMR). The enormous sensitivity enhancement afforded by optical pumping noble gases can be exploited to permit a variety of novel NMR experiments across many disciplines. Many such experiments are reviewed, including the void-space imaging of organisms and materials, NMR and MRI of living tissues, probing structure and dynamics of molecules in solution and on surfaces, and zero-field NMR and MRI

  14. Nuclear magnetic resonance of laser-polarized noble gases in molecules, materials and organisms

    Energy Technology Data Exchange (ETDEWEB)

    Goodson, Boyd McLean [Univ. of California, Berkeley, CA (United States)

    1999-12-01

    Conventional nuclear magnetic resonance (NMR) spectroscopy and magnetic resonance imaging (MRI) are fundamentally challenged by the insensitivity that stems from the ordinarily low spin polarization achievable in even the strongest NMR magnets. However, by transferring angular momentum from laser light to electronic and nuclear spins, optical pumping methods can increase the nuclear spin polarization of noble gases by several orders of magnitude, thereby greatly enhancing their NMR sensitivity. This dissertation is primarily concerned with the principles and practice of optically pumped nuclear magnetic resonance (OPNMR). The enormous sensitivity enhancement afforded by optical pumping noble gases can be exploited to permit a variety of novel NMR experiments across many disciplines. Many such experiments are reviewed, including the void-space imaging of organisms and materials, NMR and MRI of living tissues, probing structure and dynamics of molecules in solution and on surfaces, and zero-field NMR and MRI.

  15. Mid infrared resonant cavity detectors and lasers with epitaxial lead-chalcogenides

    Science.gov (United States)

    Zogg, H.; Rahim, M.; Khiar, A.; Fill, M.; Felder, F.; Quack, N.

    2010-09-01

    Wavelength tunable emitters and detectors in the mid-IR wavelength region allow applications including thermal imaging and gas spectroscopy. One way to realize such tunable devices is by using a resonant cavity. By mechanically changing the cavity length with MEMS mirror techniques, the wavelengths may be tuned over a considerable range. Resonant cavity enhanced detectors (RCED) are sensitive at the cavity resonance only. They may be applied for low resolution spectroscopy, and, when arrays of such detectors are realized, as multicolour IR-FPA or "IR-AFPA", adaptive focal plane arrays. We report the first room temperature mid-IR VECSEL (vertical external cavity surface emitting laser) with a wavelength above 3 μm. The active region is just 850 nm PbSe, followed by a 2.5 pair Bragg mirror. Output power is > 10 mW at RT.

  16. A high sensitivity nanomaterial based SAW humidity sensor

    Energy Technology Data Exchange (ETDEWEB)

    Wu, T-T; Chou, T-H [Institute of Applied Mechanics, National Taiwan University, Taipei 106, Taiwan (China); Chen, Y-Y [Department of Mechanical Engineering, Tatung University, Taipei 104, Taiwan (China)], E-mail: wutt@ndt.iam.ntu.edu.tw

    2008-04-21

    In this paper, a highly sensitive humidity sensor is reported. The humidity sensor is configured by a 128{sup 0}YX-LiNbO{sub 3} based surface acoustic wave (SAW) resonator whose operating frequency is at 145 MHz. A dual delay line configuration is realized to eliminate external temperature fluctuations. Moreover, for nanostructured materials possessing high surface-to-volume ratio, large penetration depth and fast charge diffusion rate, camphor sulfonic acid doped polyaniline (PANI) nanofibres are synthesized by the interfacial polymerization method and further deposited on the SAW resonator as selective coating to enhance sensitivity. The humidity sensor is used to measure various relative humidities in the range 5-90% at room temperature. Results show that the PANI nanofibre based SAW humidity sensor exhibits excellent sensitivity and short-term repeatability.

  17. NUMERICAL SIMULATION OF Q-SWITCHED Nd: YAG LASER WITH UNSTABLE RESONATOR AND OUTPUT VARIABLE REFLECTIVITY MIRROR

    Directory of Open Access Journals (Sweden)

    I. N. Dubinkin

    2017-05-01

    Full Text Available The article deals with a method of numerical simulation of laser oscillation in the radially symmetric unstable resonator with an output variable reflectivity mirror (VRM. Research results of the VRM parameters influence on the spatial and energy properties of the laser radiation are obtained. Numerical simulation of laser oscillation in active and passive Q-switching and comparative analysis of the spatial and energy radiation characteristics is done for these modes.

  18. Resonance absorption spectroscopy for laser-ablated lanthanide atom. (1) Optimized experimental conditions for isotope-selective absorption of gadolinium (Contract research)

    International Nuclear Information System (INIS)

    Miyabe, Masabumi; Oba, Masaki; Iimura, Hideki; Akaoka, Katsuaki; Maruyama, Yoichiro; Wakaida, Ikuo; Watanabe, Kazuo

    2008-06-01

    For remote isotope analysis of low-decontaminated TRU fuel, we are developing an analytical technique on the basis of the resonance absorption spectroscopy for the laser-ablation plume. To improve isotopic selectivity and detection sensitivity of this technique, we measured absorption spectra of Gd atom with various plume production conditions (ablation laser intensity, ambient gas and its pressure) and observation conditions (transition, probe height from sample, observation timing). As a result, high resolution spectrum was obtained from the observation of slow component of the plume produced under low-pressure rare-gas ambient. The observed narrowest linewidth of about 0.85GHz was found to be close to the Doppler width estimated for Gd atom of room temperature. Furthermore, relaxation rate of higher meta-stable state was found to be higher than that of ground state, suggesting that use of the transition arising from ground state or lower meta-stable state is preferable for highly sensitive isotope analysis. (author)

  19. Low Cost, Low Power, High Sensitivity Magnetometer

    Science.gov (United States)

    2008-12-01

    which are used to measure the small magnetic signals from brain. Other types of vector magnetometers are fluxgate , coil based, and magnetoresistance...concentrator with the magnetometer currently used in Army multimodal sensor systems, the Brown fluxgate . One sees the MEMS fluxgate magnetometer is...Guedes, A.; et al., 2008: Hybrid - LOW COST, LOW POWER, HIGH SENSITIVITY MAGNETOMETER A.S. Edelstein*, James E. Burnette, Greg A. Fischer, M.G

  20. Modelling of a diode laser with a resonant grating of quantum wells and an external mirror

    International Nuclear Information System (INIS)

    Vysotskii, D V; Elkin, N N; Napartovich, A P; Kozlovskii, Vladimir I; Lavrushin, B M

    2011-01-01

    A three-dimensional numerical model of a diode laser with a resonant grating of quantum wells (QWs) and an external mirror is developed and used to calculate diode laser pulses that are long compared to the time of reaching a stationary regime and are short enough to neglect heating of the medium. The consistent solutions of the Helmholtz field equation and the system of diffusion equations for inversion in each QW are found. A source of charge carriers can be both an electron beam and a pump laser beam. The calculations yielded the longitudinal and radial profiles of the generated field, as well as its wavelength and power. The effective threshold pump current is determined. In the created iteration algorithm, the calculation time linearly increases with the number of QWs, which allows one to find the characteristics of lasers with a large number of QWs. The output powers and beam divergence angles of a cylindrical laser are calculated for different cavity lengths and pump spot radii. After calculating the fundamental mode characteristics, high-order modes were additionally calculated on the background of the frozen carrier distributions in the QW grating. It is shown that all the competing modes remain below the excitation threshold for the pump powers used in the experiment. The calculated and experimental data for the case of pumping by a nanosecond electron beam are qualitatively compared.

  1. Vibronic Rabi resonances in harmonic and hard-wall ion traps for arbitrary laser intensity and detuning

    International Nuclear Information System (INIS)

    Lizuain, I.; Muga, J. G.

    2007-01-01

    We investigate laser-driven vibronic transitions of a single two-level atomic ion in harmonic and hard-wall traps. In the Lamb-Dicke regime, for tuned or detuned lasers with respect to the internal frequency of the ion, and weak or strong laser intensities, the vibronic transitions occur at well-isolated Rabi resonances, where the detuning-adapted Rabi frequency coincides with the transition frequency between vibrational modes. These vibronic resonances are characterized as avoided crossings of the dressed levels (eigenvalues of the full Hamiltonian). Their peculiarities due to symmetry constraints and trapping potential are also examined

  2. Computational code in atomic and nuclear quantum optics: Advanced computing multiphoton resonance parameters for atoms in a strong laser field

    Science.gov (United States)

    Glushkov, A. V.; Gurskaya, M. Yu; Ignatenko, A. V.; Smirnov, A. V.; Serga, I. N.; Svinarenko, A. A.; Ternovsky, E. V.

    2017-10-01

    The consistent relativistic energy approach to the finite Fermi-systems (atoms and nuclei) in a strong realistic laser field is presented and applied to computing the multiphoton resonances parameters in some atoms and nuclei. The approach is based on the Gell-Mann and Low S-matrix formalism, multiphoton resonance lines moments technique and advanced Ivanov-Ivanova algorithm of calculating the Green’s function of the Dirac equation. The data for multiphoton resonance width and shift for the Cs atom and the 57Fe nucleus in dependence upon the laser intensity are listed.

  3. Semi-analytical model of laser resonance absorption in plasmas with a parabolic density profile

    International Nuclear Information System (INIS)

    Pestehe, S J; Mohammadnejad, M

    2010-01-01

    Analytical expressions for mode conversion and resonance absorption of electromagnetic waves in inhomogeneous, unmagnetized plasmas are required for laboratory and simulation studies. Although most of the analyses of this problem have concentrated on the linear plasma density profile, there are a few research works that deal with different plasma density profiles including the parabolic profile. Almost none of them could give clear analytical formulae for the electric and magnetic components of the electromagnetic field propagating through inhomogeneous plasmas. In this paper, we have considered the resonant absorption of laser light near the critical density of plasmas with parabolic electron density profiles followed by a uniform over-dense region and have obtained expressions for the electric and magnetic vectors of laser light propagating through the plasma. An estimation of the fractional absorption of laser energy has also been carried out. It has been shown that, in contrast to the linear density profile, the energy absorption depends explicitly on the value of collision frequency as well as on a new parameter, N, called the over-dense density order.

  4. Jones matrix formulation of a Porro prism laser resonator with waveplates: theoretical and experimental analysis

    Science.gov (United States)

    Agrawal, L.; Bhardwaj, A.; Pal, S.; Kumar, A.

    2007-11-01

    This article presents the results of a detailed theoretical and experimental analysis carried out on a folded Z-shaped polarization coupled, electro-optically Q-switched laser resonator with Porro prisms and waveplates. The advantages of adding waveplates in a Porro prism resonator have been explored for creating high loss condition prior to Q-switching and obtaining variable reflectivity with fixed orientation of Porro prism. Generalized expressions have been derived in terms of azimuth angles and phase shifts introduced by the polarizing elements. These expressions corroborate with known reported results under appropriate substitutions. A specific case of a crossed Porro prism diode-pumped Nd:YAG laser has been theoretically and experimentally investigated. In the feedback arm, a 0.57λ waveplate oriented at 135° completely compensates the phase shift of a fused silica Porro prism and provides better tolerances than a BK-7 prism/0.60λ waveplate combination to stop prelasing. The fused silica prism/0.57λ combination with waveplate at 112° acts like a 100% mirror and was utilized for optimization of free running performance. The effective reflectivity was determined for various orientations of the quarter waveplate in the gain arm to numerically estimate the Q-switched laser pulse parameters through rate equation analysis. Experimental results match well with the theoretical analysis.

  5. Development of Laser-Polarized Noble Gas Magnetic Resonance Imaging (MRI) Technology

    Science.gov (United States)

    Walsworth, Ronald L.

    2004-01-01

    We are developing technology for laser-polarized noble gas nuclear magnetic resonance (NMR), with the aim of enabling it as a novel biomedical imaging tool for ground-based and eventually space-based application. This emerging multidisciplinary technology enables high-resolution gas-space magnetic resonance imaging (MRI)-e.g., of lung ventilation, perfusion, and gas-exchange. In addition, laser-polarized noble gases (3He and 1BXe) do not require a large magnetic field for sensitive NMR detection, opening the door to practical MRI with novel, open-access magnet designs at very low magnetic fields (and hence in confined spaces). We are pursuing two specific aims in this technology development program. The first aim is to develop an open-access, low-field (less than 0.01 T) instrument for MRI studies of human gas inhalation as a function of subject orientation, and the second aim is to develop functional imaging of the lung using laser-polarized He-3 and Xe-129.

  6. A pulsated weak-resonant-cavity laser diode with transient wavelength scanning and tracking for injection-locked RZ transmission.

    Science.gov (United States)

    Lin, Gong-Ru; Chi, Yu-Chieh; Liao, Yu-Sheng; Kuo, Hao-Chung; Liao, Zhi-Wang; Wang, Hai-Lin; Lin, Gong-Cheng

    2012-06-18

    By spectrally slicing a single longitudinal-mode from a master weak-resonant-cavity Fabry-Perot laser diode with transient wavelength scanning and tracking functions, the broadened self-injection-locking of a slave weak-resonant-cavity Fabry-Perot laser diode is demonstrated to achieve bi-directional transmission in a 200-GHz array-waveguide-grating channelized dense-wavelength-division-multiplexing passive optical network system. Both the down- and up-stream slave weak-resonant-cavity Fabry-Perot laser diodes are non-return-to-zero modulated below threshold and coherently injection-locked to deliver the pulsed carrier for 25-km bi-directional 2.5 Gbits/s return-to-zero transmission. The master weak-resonant-cavity Fabry-Perot laser diode is gain-switched at near threshold condition and delivers an optical coherent pulse-train with its mode linewidth broadened from 0.2 to 0.8 nm by transient wavelength scanning, which facilitates the broadband injection-locking of the slave weak-resonant-cavity Fabry-Perot laser diodes with a threshold current reducing by 10 mA. Such a transient wavelength scanning induced spectral broadening greatly releases the limitation on wavelength injection-locking range required for the slave weak-resonant-cavity Fabry-Perot laser diode. The theoretical modeling and numerical simulation on the wavelength scanning and tracking effects of the master and slave weak-resonant-cavity Fabry-Perot laser diodes are performed. The receiving power sensitivity for back-to-back transmission at bit-error-rate transmission is less than 2 dB for all 16 channels.

  7. Effect of self-focusing on resonant third harmonic generation of laser in a rippled density plasma

    International Nuclear Information System (INIS)

    Kaur, Sukhdeep; Sharma, A. K.; Yadav, Sushila

    2010-01-01

    Resonant third harmonic generation by a Gaussian laser beam in a rippled density plasma is studied. The laser ponderomotive force induces second harmonic longitudinal velocity on electrons that couples with the static density ripple to produce a density perturbation at 2ω,2k+q, where ω and k are the frequency and wave number of the laser and q is the ripple wave number of the laser. This density perturbation beats with electron oscillatory velocity at ω,k-vector to produce a nonlinear current driving the third harmonic generation. In the regime of quadratic nonlinearity, the self-focusing of the laser enhances the third harmonic power. However, at higher intensity, plasma density is significantly reduced on the axis, detuning the third harmonic resonance and weakening the harmonic yield. Self-focusing causes enhancement in the efficiency of harmonic generation.

  8. Review of high-sensitivity Radon studies

    Science.gov (United States)

    Wojcik, M.; Zuzel, G.; Simgen, H.

    2017-10-01

    A challenge in many present cutting-edge particle physics experiments is the stringent requirements in terms of radioactive background. In peculiar, the prevention of Radon, a radioactive noble gas, which occurs from ambient air and it is also released by emanation from the omnipresent progenitor Radium. In this paper we review various high-sensitivity Radon detection techniques and approaches, applied in the experiments looking for rare nuclear processes happening at low energies. They allow to identify, quantitatively measure and finally suppress the numerous sources of Radon in the detectors’ components and plants.

  9. Nanoimprinted polymer lasers with threshold below 100 W/cm2 using mixed-order distributed feedback resonators.

    Science.gov (United States)

    Wang, Yue; Tsiminis, Georgios; Kanibolotsky, Alexander L; Skabara, Peter J; Samuel, Ifor D W; Turnbull, Graham A

    2013-06-17

    Organic semiconductor lasers were fabricated by UV-nanoimprint lithography with thresholds as low as 57 W/cm(2) under 4 ns pulsed operation. The nanoimprinted lasers employed mixed-order distributed feedback resonators, with second-order gratings surrounded by first-order gratings, combined with a light-emitting conjugated polymer. They were pumped by InGaN LEDs to produce green-emitting lasers, with thresholds of 208 W/cm(2) (102 nJ/pulse). These hybrid lasers incorporate a scalable UV-nanoimprint lithography process, compatible with high-performance LEDs, therefore we have demonstrated a coherent, compact, low-cost light source.

  10. Effect of the background radiation of a copper vapor laser with an unstable resonator on dye lasing

    Energy Technology Data Exchange (ETDEWEB)

    Elaev, V F; Mirza, S M; Sukhanov, V B; Troitskii, V O; Soldatov, A N

    1986-05-01

    Results of an experimental study of the emission divergence of a copper vapor laser with an unstable resonator are reported. It is shown that a copper vapor laser beam can be conveniently treated as a pair of components with a divergence higher or lower than a certain optimal value; the percent ratio of the components varies with the pulse repetition frequency. In the case where a copper vapor laser is used to pump a dye laser, the contribution of the component with the higher divergence to dye lasing does not exceed 1 percent. 7 references.

  11. Resonantly diode pumped Er:YAG laser systems emitting at 1645 nm for methane detection

    International Nuclear Information System (INIS)

    Fritsche, H; Lux, O; Wang, X; Zhao, Z; Eichler, H J

    2013-01-01

    We report on the development of compact and frequency-stable Er:YAG laser systems emitting in the eye-safe spectral region. Resonant cw diode pumping provides 4.5 W output power in cw operation and 2.2 mJ in Q-switched operation with pulse duration of about 140 ns. The application of intra-cavity etalons allows for wavelength tuning from 1645.22 to 1646.33 nm while the frequency stability accounts for less than 50 MHz. The potential of the erbium laser sources in terms of methane detection was evaluated under laboratory conditions by absorption measurements employing a multi-pass absorption cell. The experimental investigations were accompanied by theoretical studies on the influence of pressure broadening on the absorption behavior of methane. (letter)

  12. Stochastic resonance for signal-modulated pump noise in a single-mode laser

    Institute of Scientific and Technical Information of China (English)

    Liangying Zhang; Li Cao; Fahui Zhu

    2006-01-01

    By adopting the gain-noise model of the single-mode laser in which with bias and periodical signals serve as inputs, combining with the effect of coloured pump noise, we use the linear approximation method to calculate the power spectrum and signal-to-noise ratio (SNR) of the laser intensity under the condition of pump noise and quantum noise cross-related in the form of δ function. It is found that with the change of pump noise correlation time, both SNR and the output power will occur stochastic resonance (SR). If the bias signal α is very small, changing the intensities of pump noise and quantum noise respectively does not lead to the appearance of SR in the SNR; while α increases to a certain number, SR appears.

  13. Terahertz lasers and amplifiers based on resonant optical phonon scattering to achieve population inversion

    Science.gov (United States)

    Williams, Benjamin S. (Inventor); Hu, Qing (Inventor)

    2009-01-01

    The present invention provides quantum cascade lasers and amplifier that operate in a frequency range of about 1 Terahertz to about 10 Terahertz. In one aspect, a quantum cascade laser of the invention includes a semiconductor heterostructure that provides a plurality of lasing modules connected in series. Each lasing module includes a plurality of quantum well structure that collectively generate at least an upper lasing state, a lower lasing state, and a relaxation state such that the upper and the lower lasing states are separated by an energy corresponding to an optical frequency in a range of about 1 to about 10 Terahertz. The lower lasing state is selectively depopulated via resonant LO-phonon scattering of electrons into the relaxation state.

  14. Bistable output from a coupled-resonator vertical-cavity laser diode

    International Nuclear Information System (INIS)

    Fischer, A. J.; Choquette, K. D.; Chow, W. W.; Allerman, A. A.; Geib, K.

    2000-01-01

    We report a monolithic coupled-resonator vertical-cavity laser with an ion-implanted top cavity and a selectively oxidized bottom cavity which exhibits bistable behavior in the light output versus injection current. Large bistability regions over current ranges as wide as 18 mA have been observed with on/off contrast ratios of greater than 20 dB. The position and width of the bistability region can be varied by changing the bias to the top cavity. Switching between on and off states can be accomplished with changes as small as 250 μW to the electrical power applied to the top cavity. The bistable behavior is the response of the nonlinear susceptibility in the top cavity to the changes in the bottom intracavity laser intensity as the bottom cavity reaches the thermal rollover point

  15. Study of Low Work Function Materials for Hot Cavity Resonance Ionization Laser Ion Sources

    CERN Document Server

    Catherall, R; Fedosseev, V; Marsh, B; Mattolat, C; Menna, Mariano; Österdahl, F; Raeder, S; Schwellnus, F; Stora, T; Wendt, K; CERN. Geneva. AB Department

    2008-01-01

    The selectivity of a hot cavity resonance ionization laser ion source (RILIS) is most often limited by contributions from competing surface ionization on the hot walls of the ionization cavity. In this article we present investigations on the properties of designated high-temperature, low-work function materials regarding their performance and suitability as cavity material for RILIS. Tungsten test cavities, impregnated with a mixture of barium oxide and strontium oxide (BaOSrO on W), or alternatively gadolinium hexaboride (GdB6) were studied in comparison to a standard tungsten RILIS cavity as being routinely used for hot cavity laser ionization at ISOLDE. Measurement campaigns took place at the off-line mass separators at ISOLDE / CERN, Geneva and RISIKO / University of Mainz.

  16. Study of low work function materials for hot cavity resonance ionization laser ion sources

    CERN Document Server

    Schwellnus, F; Crepieux, B; Fedosseev, V N; Marsh, B A; Mattolat, Ch; Menna, M; Österdahl, F K; Raeder, S; Stora, T; Wendta, K

    2009-01-01

    The selectivity of a hot cavity resonance ionization laser ion source (RILIS) is most often limited by contributions from competing surface ionization of the hot walls of the ionization cavity. In this article we present investigations on the properties of designated high temperature, low work function materials regarding their performance and suitability as cavity material for RILIS. Tungsten test cavities, impregnated with a mixture of barium oxide and strontium oxide (BaOSrO on W), or alternatively gadolinium hexaboride (GdB6) were studied in comparison to a standard tungsten RILIS cavity as being routinely used for hot cavity laser ionization at ISOLDE. Measurement campaigns took place at the off-line mass separators at ISOLDE/CERN, Geneva and RISIKO/University of Mainz.

  17. Hybrid lasers produced in potassium vapor by off-resonance pumping

    International Nuclear Information System (INIS)

    Clark, B.K.; Stack, C.A.; Muehsler, H.E.

    1993-01-01

    Pulsed amplified emissions are observed at or near atomic transitions cascading down from the K(6S) and K(4D 5/2 ) states, when a pulsed dye laser is tuned near the K(6S left-arrow 4 3/2,1/2 ) and the K(4D 5/2 left-arrow 4P 3/2 ) transitions. Emissions are suppressed when the pulsed dye laser is tuned to the K(4D 3/2 left-arrow 4P 5/3,3/2 ) transitions. The pulsed dye laser is used to excite molecules in a heat-pipe oven from high-bring ro-vibrational levels in the K 2 (X 1 Σ g + ) ground state to ro-vibrational levels in the K 2 (B 1 product u ) state that predissociate to K(4S) and K(4P) atoms. The transitions can be pumped when the laser is tuned sufficiently close to the atomic resonances. We discuss the non-linear mechanisms responsible for the observed emissions. Emissions cascading down from the K(4S) state were first reported by Wang et al

  18. Resonant photoacoustic detection of NO2 traces with a Q-switched green laser

    Science.gov (United States)

    Slezak, Verónica; Codnia, Jorge; Peuriot, Alejandro L.; Santiago, Guillermo

    2003-01-01

    Resonant photoacoustic detection of NO2 traces by means of a high repetition pulsed green laser is presented. The resonator is a cylindrical Pyrex glass cell with a measured Q factor 380 for the first radial mode in air at atmospheric pressure. The system is calibrated with known mixtures in dry air and a minimum detectable volume concentration of 50 parts in 109 is obtained (S/N=1). Its sensitivity allows one to detect and quantify NO2 traces in the exhaust gases of cars. Previously, the analysis of gas adsorption and desorption on the walls and of changes in the sample composition is carried out in order to minimize errors in the determination of NO2 content upon application of the extractive method. The efficiency of catalytic converters of several models of automobiles is studied and the NO2 concentration in samples from exhausts of different types of engine (gasoline, diesel, and methane gas) at idling operation are measured.

  19. Above-threshold ionization of atoms by resonant XUV laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Rodriguez, V D [Departamento de Fisica and IFIBA-CONICET, FCEyN, Universidad de Buenos Aires, 1428 Buenos Aires (Argentina); Arbo, D G [Instituto de AstronomIa y Fisica del Espacio, FCEN-UBA CONICET, CC 67 Suc 28 Buenos Aires (Argentina); Macri, P A, E-mail: vladimir@df.uba.ar [Departamento de Fisica, FCEyN, Instituto de Investigaciones Fisicas de Mar del Plata (IFIMAR), Universidad Nacional de Mar del Plata-CONICET, Funes 3350, 7600 Mar del Plata (Argentina)

    2011-06-28

    Above-threshold ionization of atoms by XUV short laser pulses with frequencies close to the resonant 1s-2p transition is investigated. We present a theory based on a variational expression using trial wavefunctions for the final and the initial states. For the former we use a Coulomb-Volkov wavefunction, and for the latter a close-coupling solution of the time-dependent Schroedinger equation considering a few bound states. The close-coupling Coulomb-Volkov theory, fully accounting for the important 1s-2p transition, explains the photoelectron spectrum as well as the total ionization cross sections for the resonant case. We also compare the partial wave populations and angular distributions given by the theory with the numerical solutions of the time-dependent Schroedinger equation.

  20. Laser deposition of resonant silicon nanoparticles on perovskite for photoluminescence enhancement

    Science.gov (United States)

    Tiguntseva, E. Y.; Zalogina, A. S.; Milichko, V. A.; Zuev, D. A.; Omelyanovich, M. M.; Ishteev, A.; Cerdan Pasaran, A.; Haroldson, R.; Makarov, S. V.; Zakhidov, A. A.

    2017-11-01

    Hybrid lead halide perovskite based optoelectronics is a promising area of modern technologies yielding excellent characteristics of light emitting diodes and lasers as well as high efficiencies of photovoltaic devices. However, the efficiency of perovskite based devices hold a potential of further improvement. Here we demonstrate high photoluminescence efficiency of perovskites thin films via deposition of resonant silicon nanoparticles on their surface. The deposited nanoparticles have a number of advances over their plasmonic counterparts, which were applied in previous studies. We show experimentally the increase of photoluminescence of perovskite film with the silicon nanoparticles by 150 % as compared to the film without the nanoparticles. The results are supported by numerical calculations. Our results pave the way to high throughput implementation of low loss resonant nanoparticles in order to create highly effective perovskite based optoelectronic devices.

  1. b-dipole transitions in trans-HOCO observed by far infrared laser magnetic resonance

    International Nuclear Information System (INIS)

    Sears, T.J.; Radford, H.E.; Moore, M.A.

    1993-01-01

    Far infrared laser magnetic resonance spectroscopy is used to measure components of 12 rotational transitions in the ground state of the HOCO radical. The transitions are all b-dipole in character in contrast to the a-dipole rotational spectrum previously reported [Radford, Wei, and Sears, J. Chem. Phys. 97, 3989 (1992)]. The new data determine the A rotational constant to high precision and allow the determination of several centrifugal distortion constants for the first time. The hyperfine coupling in the radical leads to observable splittings in several of the observed transitions and these are used to estimate two of the four expected nonzero hyperfine parameters in the radical

  2. Resonance enhanced laser mass spectrometry for process- and environmental-analysis: Applications and perspectives

    International Nuclear Information System (INIS)

    Zimmermann, Ralf; Dorfner, Ralph; Kettrup, Antonius; Heger, Hans Joerg; Boesl, Ulrich

    1998-01-01

    Laser induced Resonance-Enhanced Multi-Photon Ionization Time-Of-Flight Mass Spectrometry (REMPI TOFMS) is a highly selective as well as sensitive analytical technique, well suited for species selective, on-line monitoring of trace-substances. In this contribution some analytical applications of a mobile REMPI-TOFMS are presented. This includes REMPI-TOMS on-line analysis of coffee roasting gas and waste incineration flue gas as well as headspace measurements of pulp processing lye or rapid analysis of polycyclic aromatic hydrocarbons from soil samples via thermal desorption

  3. Laser-excited Fluorescence And Electron-spin Resonance Of Er3+ In Polycrystalline Alcl3

    OpenAIRE

    Ceotto G.; Pires M.A.; Sanjurjo J.A.; Rettori C.; Barberis G.E.

    1990-01-01

    The green fluorescence transitions among the levels corresponding to the 4S3/2 and 4I15/2 configurations of Er3+ diluted in AlCl3 have been measured using laser excitation. The data allow us to determine the crystalline-field splittings of these levels and, in turn, the spin-Hamiltonian parameters. The electron-paramagnetic-resonance spectrum observed at low temperatures is in good agreement with that expected from these parameters. © 1990 The American Physical Society.

  4. Effects of frequency mismatch on a self-consistent arbitrary amplitude cyclotron resonance laser accelerator

    International Nuclear Information System (INIS)

    Pakter, R.; Schneider, R.S.; Rizzato, F.B.

    1993-01-01

    The cyclotron-resonance laser accelerator (CRLA), where a coherent electromagnetic wave may transfer a large amount of energy to a beam of electrons gravitating in a guide magnetic field is studied. This large amount of transferred energy takes place due to the autoresonance mechanism where, under some ideal conditions, an initial wave-particle synchronism is self-sustained throughout the accelerating period. An improved analysis of the mentioned self-consistent wave-particle interaction, taking into account a possible frequency mismatch between wave and particles. It is also shown how the frequency mismatch can compensate the dispersion effects. (L.C.J.A.)

  5. Measurement of changes in nuclear charge radii of 2r by laser-induced resonance fluorescence

    International Nuclear Information System (INIS)

    Gangrskij, Yu.P.; Zemlyanoj, S.G.; Marinova, K.P.; Markov, B.N.; Khoang Tkhi Kim Khueh; Chan Kong Tam; Kul'dzhanov, B.K.

    1987-01-01

    The optical isotopic shifts of Zr stable isotopes have been measured in three atomic transitions of type 4d 2 5s 2 → 4d 2 5s5p using the technique of laser-induced resonance fluorescence. The changes of nuclear mean-square charge radius Δ 2 > have been determined. The extracted values of Δ 2 > are compared to predictions of the droplet model. It is shown that the droplet model calculations can be made to agree with the experimental results, if changes of nuclear dynamical octupole deformation and of surface diffuseness parameter are taken into account

  6. Limiting effects on laser compression by resonant backward Raman scattering in modern experiments

    International Nuclear Information System (INIS)

    Yampolsky, Nikolai A.; Fisch, Nathaniel J.

    2011-01-01

    Through resonant backward Raman scattering, the plasma wave mediates the energy transfer between long pump and short seed laser pulses. These mediations can result in pulse compression at extraordinarily high powers. However, both the overall efficiency of the energy transfer and the duration of the amplified pulse depend upon the persistence of the plasma wave excitation. At least with respect to the recent state-of-the-art experiments, it is possible to deduce that at present the experimentally realized efficiency of the amplifier is likely constrained mainly by two effects, namely, the pump chirp and the plasma wave wavebreaking.

  7. Musical instrument pickup based on a laser locked to an optical fiber resonator.

    Science.gov (United States)

    Avino, Saverio; Barnes, Jack A; Gagliardi, Gianluca; Gu, Xijia; Gutstein, David; Mester, James R; Nicholaou, Costa; Loock, Hans-Peter

    2011-12-05

    A low-noise transducer based on a fiber Fabry-Perot (FFP) cavity was used as a pickup for an acoustic guitar. A distributed feedback (DFB) laser was locked to a 25 MHz-wide resonance of the FFP cavity using the Pound-Drever-Hall method. The correction signal was used as the audio output and was preamplified and sampled at up to 96 kHz. The pickup system is largely immune against optical noise sources, exhibits a flat frequency response from the infrasound region to about 25 kHz, and has a distortion-free audio output range of about 50 dB.

  8. 4d--4f emission resonances in laser-produced plasmas

    International Nuclear Information System (INIS)

    O'Sullivan, G.; Carroll, P.K.

    1981-01-01

    Using targets containing compounds of the elements cesium through lutetium, we studied the spectra of laser-produced plasmas in the grazing-incidence region from 40 to 200 A. The spectra are characterized by strong regions of resonancelike emission extending typically over 9--18 eV. With increasing Z, the spectra show certain systematic variations in character and move monotonically toward shorter wavelengths. From a collisional-radiative plasma model, the ion stages responsible for the emision are identified as VIII through XVI. The resonances are attributed to 4-4f transitions that, because Dn = 0, tend to overlap for different ion stages of the same element

  9. First observation of laser-induced resonant annihilation in metastable antiprotonic helium atoms

    International Nuclear Information System (INIS)

    Morita, N.; Kumakura, M.; Yamazaki, T.

    1993-11-01

    We have observed the first laser-induced resonant transitions in antiprotonic helium atoms. These occur between metastable states and Auger dominated short lived states, and show that the anomalous longevity of antiprotons previously observed in helium media results from the formation of high-n high-l atomic states of p-barHe + . The observed transition with vacuum wavelength 597.259 ± 0.002 nm and lower-state lifetime 15 ± 1 ns is tentatively assigned to (n,l) = (39,35) → (38,34). (author)

  10. Laser-ultrasound spectroscopy apparatus and method with detection of shear resonances for measuring anisotropy, thickness, and other properties

    Science.gov (United States)

    Levesque, Daniel; Moreau, Andre; Dubois, Marc; Monchalin, Jean-Pierre; Bussiere, Jean; Lord, Martin; Padioleau, Christian

    2000-01-01

    Apparatus and method for detecting shear resonances includes structure and steps for applying a radiation pulse from a pulsed source of radiation to an object to generate elastic waves therein, optically detecting the elastic waves generated in the object, and analyzing the elastic waves optically detected in the object. These shear resonances, alone or in combination with other information, may be used in the present invention to improve thickness measurement accuracy and to determine geometrical, microstructural, and physical properties of the object. At least one shear resonance in the object is detected with the elastic waves optically detected in the object. Preferably, laser-ultrasound spectroscopy is utilized to detect the shear resonances.

  11. Peculiarities of the fundamental mode structure in stable-resonator lasers upon spatially inhomogeneous amplification

    International Nuclear Information System (INIS)

    Gorbunkov, Mikhail V; Kostryukov, P V; Telegin, L S; Tunkin, V G; Yakovlev, D V

    2007-01-01

    The structure of the fundamental mode of a laser is calculated by the iteration Fox-Li method in the case of inhomogeneous unsaturated amplification produced by axially symmetric longitudinal pumping. The calculation is performed for different parameters g 1 and g 2 of the resonator within the entire stability region. It is shown that in the case of inhomogeneous amplification, the fundamental mode considerably deviates from the Gaussian mode of an empty resonator only in the so-called critical configurations of the resonator, when the quantity [arccos(g 1 g 2 ) 1/2 ]/π is zero or takes a number of values expressed by irreducible fractions m/n. For the Fresnel number N F = 9, configurations with m/n = 1/2, 2/5, 3/8, 1/3, 3/10, 1/4, 1/5, 1/6, 1/8, and 1/10 are pronounced. As N F increases, the number of critical configurations increases. The expansion in a system of Laguerre-Gaussian beams shows that the fundamental mode in critical configurations is formed by a set of beams with certain radial indices p phased in the active medium. (resonators. modes)

  12. Far off-resonance laser frequency stabilization using multipass cells in Faraday rotation spectroscopy.

    Science.gov (United States)

    Quan, Wei; Li, Yang; Li, Rujie; Shang, Huining; Fang, Zishan; Qin, Jie; Wan, Shuangai

    2016-04-01

    We propose a far off-resonance laser frequency stabilization method by using multipass cells in Rb Faraday rotation spectroscopy. Based on the detuning equation, if multipass cells with several meters optical path length are used in the conventional Faraday spectroscopy, the detuning of the lock point can be extended much further from the alkali metal resonance. A plate beam splitter was used to generate two different Faraday signals at the same time. The transmitted optical path length was L=50  mm and the reflected optical path length was 2L=100  mm. When the optical path length doubled, the detuning of the lock points moved further away from the atomic resonance. The temperature dependence of the detuning of the lock point was also analyzed. A temperature-insensitive lock point was found near resonance when the cell temperature was between 110°C and 130°C. We achieved an rms fluctuation of 0.9 MHz/23 h at a detuning of 0.5 GHz. A frequency drift of 16 MHz/h at a detuning of -5.6  GHz and 4 MHz/h at a detuning of -5.2  GHz were also obtained for the transmitted and reflected light Faraday signal.

  13. Resonant ionization by laser beams: application to ions sources and to study the nuclear structure of radioactive tellurium isotopes

    International Nuclear Information System (INIS)

    Sifi, R.

    2007-07-01

    The radioactive ion beams that are produced through current isotope separators are well separated according to the A mass but not according to the Z parameter. The resonant ionization through laser beams applied to ion sources allows the production of radioactive ion beam in a very selective and efficient way by eliminating the isobaric contamination. The first chapter is dedicated to the resonant ionization by laser beams, we describe the principle, the experimental setting, the lasers used, the ionization schemes and the domain of application. The second chapter deals with the application of resonant ionization to laser ion sources for the production of radioactive ion beams. We present experimental tests performed for getting copper ion beams. Resonant ionization through laser is also used in the spectroscopy experiments performed at the Isolde (isotope separation on-line device) installation in CERN where more than 20 elements are ionized very efficiently. The technique is based on a frequency scanning around the excitation transition of the atoms in order to probe the hyperfine structure. Laser spectroscopy allows the determination of the hyperfine structure as well as the isotopic shift of atoms. In the third chapter the method is applied to the spectroscopy of tellurium atoms. First, we define the 2 parameters on which the extraction is based: charge radius and nuclear moments, then we present several theoretical models that we have used to assess our experimental results. (A.C.)

  14. Efficient second harmonic generation of a diode-laser-pumped CW Nd:YAG laser using monolithic MgO:LiNbO3 external resonant cavities

    Science.gov (United States)

    Kozlovsky, William J.; Nabors, C. D.; Byer, Robert L.

    1988-01-01

    56-percent efficient external-cavity-resonant second-harmonic generation of a diode-laser pumped, CW single-axial-mode Nd:YAG laser is reported. A theory of external doubling with a resonant fundamental is presented and compared to experimental results for three monolithic cavities of nonlinear MgO:LiNbO3. The best conversion efficiency was obtained with a 12.5-mm-long monolithic ring cavity doubler, which produced 29.7 mW of CW, single-axial model 532-nm radiation from an input of 52.5 mW.

  15. High sensitivity optical molecular imaging system

    Science.gov (United States)

    An, Yu; Yuan, Gao; Huang, Chao; Jiang, Shixin; Zhang, Peng; Wang, Kun; Tian, Jie

    2018-02-01

    Optical Molecular Imaging (OMI) has the advantages of high sensitivity, low cost and ease of use. By labeling the regions of interest with fluorescent or bioluminescence probes, OMI can noninvasively obtain the distribution of the probes in vivo, which play the key role in cancer research, pharmacokinetics and other biological studies. In preclinical and clinical application, the image depth, resolution and sensitivity are the key factors for researchers to use OMI. In this paper, we report a high sensitivity optical molecular imaging system developed by our group, which can improve the imaging depth in phantom to nearly 5cm, high resolution at 2cm depth, and high image sensitivity. To validate the performance of the system, special designed phantom experiments and weak light detection experiment were implemented. The results shows that cooperated with high performance electron-multiplying charge coupled device (EMCCD) camera, precision design of light path system and high efficient image techniques, our OMI system can simultaneously collect the light-emitted signals generated by fluorescence molecular imaging, bioluminescence imaging, Cherenkov luminance and other optical imaging modality, and observe the internal distribution of light-emitting agents fast and accurately.

  16. High sensitivity troponin and valvular heart disease.

    Science.gov (United States)

    McCarthy, Cian P; Donnellan, Eoin; Phelan, Dermot; Griffin, Brian P; Enriquez-Sarano, Maurice; McEvoy, John W

    2017-07-01

    Blood-based biomarkers have been extensively studied in a range of cardiovascular diseases and have established utility in routine clinical care, most notably in the diagnosis of acute coronary syndrome (e.g., troponin) and the management of heart failure (e.g., brain-natriuretic peptide). The role of biomarkers is less well established in the management of valvular heart disease (VHD), in which the optimal timing of surgical intervention is often challenging. One promising biomarker that has been the subject of a number of recent VHD research studies is high sensitivity troponin (hs-cTn). Novel high-sensitivity assays can detect subclinical myocardial damage in asymptomatic individuals. Thus, hs-cTn may have utility in the assessment of asymptomatic patients with severe VHD who do not have a clear traditional indication for surgical intervention. In this state-of-the-art review, we examine the current evidence for hs-cTn as a potential biomarker in the most commonly encountered VHD conditions, aortic stenosis and mitral regurgitation. This review provides a synopsis of early evidence indicating that hs-cTn has promise as a biomarker in VHD. However, the impact of its measurement on clinical practice and VHD outcomes needs to be further assessed in prospective studies before routine clinical use becomes a reality. Copyright © 2017 Elsevier Inc. All rights reserved.

  17. Development of sodium leak detection technology using laser resonance ionization mass spectrometry. Design and functional test using prototype sodium detection system

    International Nuclear Information System (INIS)

    Aoyama, Takafumi; Ito, Chikara; Harano, Hideki; Okazaki, Koki; Watanabe, Kenichi; Iguchi, Tetsuo

    2009-01-01

    In a sodium-cooled fast reactor, highly sensitive technology is required to detect small amounts of sodium leaking from the cooling system piping or components. The conventional sodium leak detectors have a fundamental difficulty in improving the detection sensitivity for a sodium leak because of the presence of salinity ( 23 NaCl) in the atmosphere around the components and piping of cooling systems. In order to overcome this problem, an innovative technology has been developed to selectively detect the radioactive sodium ( 22 Na) produced by a neutron reaction in the primary cooling system using Laser Resonance Ionization Mass Spectrometry (RIMS). In this method, sodium ions produced with the two processes of (1) atomization of sodium aerosols and (2) resonance ionization of sodium atom, are detected selectively using a time-of-flight mass spectrometer. The 22 Na can be distinguished from the stable isotope ( 23 Na) by mass spectrometry, which is the advantage of RIMS comparing to the other methods. The design and the construction of the prototype system based on fundamental experiments are shown in the paper. The aerodynamic lens was newly introduced, which can transfer aerosols at atmospheric pressure into a vacuum chamber while increasing the aerosol density at the same time. Furthermore, the ionization process was applied by using the external electric field after resonance exciting from the ground level to the Rydberg level in order to increase the ionization efficiency. The preliminary test results using the stable isotope ( 23 Na) showed that prototype system could easily detect sodium aerosol of 100 ppb, equivalent to the sensitivity of the conventional detectors. (author)

  18. Deposition of Methylammonium Lead Triiodide by Resonant Infrared Matrix-Assisted Pulsed Laser Evaporation

    Science.gov (United States)

    Barraza, E. Tomas; Dunlap-Shohl, Wiley A.; Mitzi, David B.; Stiff-Roberts, Adrienne D.

    2018-02-01

    Resonant infrared matrix-assisted pulsed laser evaporation (RIR-MAPLE) was used to deposit the metal-halide perovskite (MHP) CH3NH3PbI3 (methylammonium lead triiodide, or MAPbI), creating phase-pure films. Given the moisture sensitivity of these crystalline, multi-component organic-inorganic hybrid materials, deposition of MAPbI by RIR-MAPLE required a departure from the use of water-based emulsions as deposition targets. Different chemistries were explored to create targets that properly dissolved MAPbI components, were stable under vacuum conditions, and enabled resonant laser energy absorption. Secondary phases and solvent contamination in the resulting films were studied through Fourier transform infrared (FTIR) absorbance and x-ray diffraction (XRD) measurements, suggesting that lingering excess methylammonium iodide (MAI) and low-vapor pressure solvents can distort the microstructure, creating crystalline and amorphous non-perovskite phases. Thermal annealing of films deposited by RIR-MAPLE allowed for excess solvent to be evaporated from films without degrading the MAPbI structure. Further, it was demonstrated that RIR-MAPLE does not require excess MAI to create stoichiometric films with optoelectronic properties, crystal structure, and film morphology comparable to films created using more established spin-coating methods for processing MHPs. This work marks the first time a MAPLE-related technique was used to deposit MHPs.

  19. Isotopic imaging via nuclear resonance fluorescence with laser-based Thomson radiation

    Science.gov (United States)

    Barty, Christopher P. J. [Hayward, CA; Hartemann, Frederic V [San Ramon, CA; McNabb, Dennis P [Alameda, CA; Pruet, Jason A [Brentwood, CA

    2009-07-21

    The present invention utilizes novel laser-based, high-brightness, high-spatial-resolution, pencil-beam sources of spectrally pure hard x-ray and gamma-ray radiation to induce resonant scattering in specific nuclei, i.e., nuclear resonance fluorescence. By monitoring such fluorescence as a function of beam position, it is possible to image in either two dimensions or three dimensions, the position and concentration of individual isotopes in a specific material configuration. Such methods of the present invention material identification, spatial resolution of material location and ability to locate and identify materials shielded by other materials, such as, for example, behind a lead wall. The foundation of the present invention is the generation of quasimonochromatic high-energy x-ray (100's of keV) and gamma-ray (greater than about 1 MeV) radiation via the collision of intense laser pulses from relativistic electrons. Such a process as utilized herein, i.e., Thomson scattering or inverse-Compton scattering, produces beams having diameters from about 1 micron to about 100 microns of high-energy photons with a bandwidth of .DELTA.E/E of approximately 10E.sup.-3.

  20. Temperature mapping of laser-induced hyperthermia in an ocular phantom using magnetic resonance thermography.

    Science.gov (United States)

    Maswadi, Saher M; Dodd, Stephen J; Gao, Jia-Hong; Glickman, Randolph D

    2004-01-01

    Laser-induced heating in an ocular phantom is measured with magnetic resonance thermography (MRT) using temperature-dependent phase changes in proton resonance frequency. The ocular phantom contains a layer of melanosomes isolated from bovine retinal pigment epithelium. The phantom is heated by the 806-nm output of a continuous wave diode laser with an irradiance of 2.4 to 21.6 W/cm2 in a beam radius of 0.8 or 2.4 mm, depending on the experiment. MRT is performed with a 2 T magnet, and a two-turn, 6-cm-diam, circular radio frequency coil. Two-dimensional temperature gradients are measured within the plane of the melanin layer, as well as normal to it, with a temperature resolution of 1 degrees C or better. The temperature gradients extending within the melanin layer are broader than those orthogonal to the layer, consistent with the higher optical absorption and consequent heating in the melanin. The temperature gradients in the phantom measured by MRT closely approximate the predictions of a classical heat diffusion model. Three-dimensional temperature maps with a spatial resolution of 0.25 mm in all directions are also made. Although the temporal resolution is limited in the prototype system (22.9 s for a single image "slice"), improvements in future implementations are likely. These results indicate that MRT has sufficient spatial and temperature resolution to monitor target tissue temperature during transpupillary thermotherapy in the human eye.

  1. CALDER: High-sensitivity cryogenic light detectors

    International Nuclear Information System (INIS)

    Casali, N.; Bellini, F.; Cardani, L.

    2017-01-01

    The current bolometric experiments searching for rare processes such as neutrinoless double-beta decay or dark matter interaction demand for cryogenic light detectors with high sensitivity, large active area and excellent scalability and radio-purity in order to reduce their background budget. The CALDER project aims to develop such kind of light detectors implementing phonon-mediated Kinetic Inductance Detectors (KIDs). The goal for this project is the realization of a 5 × 5 cm"2 light detector working between 10 and 100mK with a baseline resolution RMS below 20 eV. In this work the characteristics and the performances of the prototype detectors developed in the first project phase will be shown.

  2. Highly sensitive microcalorimeters for radiation research

    International Nuclear Information System (INIS)

    Avaev, V.N.; Demchuk, B.N.; Ioffe, L.A.; Efimov, E.P.

    1984-01-01

    Calorimetry is used in research at various types of nuclear-physics installations to obtain information on the quantitative and qualitative composition of ionizing radiation in a reactor core and in the surrounding layers of the biological shield. In this paper, the authors examine the characteristics of highly sensitive microcalorimeters with modular semiconductor heat pickups designed for operation in reactor channels. The microcalorimeters have a thin-walled aluminum housing on whose inner surface modular heat pickups are placed radially as shown here. The results of measurements of the temperature dependence of the sensitivity of the microcalorimeters are shown. The results of measuring the sensitivity of a PMK-2 microcalorimeter assembly as a function of integrated neutron flux for three energy intervals and the adsorbed gamma energy are shown. In order to study specimens with different shapes and sizes, microcalorimeters with chambers in the form of cylinders and a parallelepiped were built and tested

  3. High Contrast Coherent Population Trapping Resonances in Cs Vapour Cells with a Simple-Architecture Laser System

    International Nuclear Information System (INIS)

    Liu, Xiaochi

    2013-01-01

    This thesis reports the development of a simple-architecture laser system resonant at 895 nm used for the detection of high-contrast coherent population trapping (CPT) resonances in Cs vapor cells. The laser system combines a distributed feedback-diode (DFB) laser, a pigtailed Mach-Zehnder intensity electro-optic modulator (EOM) driven at 4.596 GHz for the generation of optical sidebands frequency-split by 9.192 GHz and a Michelson delay-line system to produce a bi-chromatic optical field that alternates between right and left circular polarization. This polarization pumping scheme, first proposed by Happer's group in Princeton on K atoms, allows to optically pump a maximum number of Cs atoms into the 0-0 magnetic field insensitive clock transition. Advanced noise reduction techniques were implemented in order to stabilize the laser power, the optical carrier suppression at the output of the EOM and the DFB laser frequency. Using this system, we demonstrated the detection of CPT resonances with a contrast of 80% in cm-scale Cs vapor cells. This contrast was measured to be increased until a saturation effect with the laser power at the expense of the CPT line broadening. To circumvent this issue, we proposed with a simple setup Ramsey spectroscopy of CPT resonances in vapor cells to combine high-contrast and narrow line width of the CPT resonances. In this setup, the EOM is used both for optical sidebands generation and light switch to produce Ramsey interaction. Ramsey fringes of 166 Hz line width with a contrast better than 30% were detected with this setup. This laser system will be in a near future devoted to be used for the development of a high-performance CPT-based atomic clock. (author)

  4. Stochastic resonance driven by time-modulated correlated coloured noise sources in a single-mode laser

    International Nuclear Information System (INIS)

    De-Yi, Chen; Li, Zhang

    2009-01-01

    This paper investigates the phenomenon of stochastic resonance in a single-mode laser driven by time-modulated correlated coloured noise sources. The power spectrum and signal-to-noise ratio R of the laser intensity are calculated by the linear approximation. The effects caused by noise self-correlation time τ 1 , τ 2 and cross-correlated time τ 3 for stochastic resonance are analysed in two ways: τ 1 , τ 2 and τ 3 are taken to be the independent variables and the parameters respectively. The effects of the gain coefficient Γ and loss coefficient K on the stochastic resonance are also discussed. It is found that besides the presence of the standard form and the broad sense of stochastic resonance, the number of extrema in the curve of R versus K is reduced with the increase of the gain coefficient Γ

  5. Resonant multiphoton ionization of caesium atoms by ultra-short laser pulses at 1.06 μm

    International Nuclear Information System (INIS)

    Lompre, L.A.; Mainfray, G.; Manus, C.; Thebault, J.

    1978-01-01

    This paper reports the four-photon ionization of caesium atoms when the laser frequency is tuned through the resonant three-photon transition 6S → 6F. This experiment was performed by using a tunable-wavelength bandwidth-limited subnanosecond laser pulse at 1.06 μm, in the 10 8 -10 9 W.cm -2 laser intensity range. Pulse widths of 1.5 ns, 50 ps, and 15 ps were used. The resonant character of the multiphoton ionization process was observed, even with the shortest pulse of 15 ps. Nevertheless the influence of a temporal effect is demonstrated according to theoretical predictions. The resonance shift ΔE of the 6S → 6F transition energy was found to be linear with the laser intensity I within the range 10 8 -10 9 W.cm -2 . ΔE = αI, with α = 2 cm -1 /GW.cm -2 . This results confirms previous measurements performed with single-mode 35 ns laser pulses and is in very good agreement with calculated resonance shifts

  6. Analysis of 81Kr in groundwater using laser resonance ionization spectroscopy

    International Nuclear Information System (INIS)

    Kramer, S.D.; Hurst, G.S.; Chen, C.H.

    1985-10-01

    A new analytical technique based on resonant ionization of krypton with a vacuum ultraviolet (VUV) laser source was used to determine low-level 81 Kr concentrations in groundwater. The long half-life (210,000 years) and low concentration (1.3 x 10 3 81 Kr atoms per liter of modern water at 10 0 C) make the detection of 81 Kr by radioactive counting techniques extremely difficult. In this method, krypton gas was removed from water taken from an underground Swiss aquifer using standard cryogenic and chromatographic techniques. Stable krypton isotopes were then reduced by a factor of 10 7 by a two-stage isotopic enrichment cycle using a commercially available mass spectrometer. The enriched gas containing about 10 8 stable krypton atoms and about 10 3 atoms of 81 Kr was implanted into a silicon disc. This disc was then placed in the high vacuum final counting chamber and the krypton was released by laser annealing. This chamber contained a quadrupole mass spectrometer which used a pulsed VUV laser source as the ionizer. The measured signal indicated that the sample contained 1200 (+-300) atoms of 81 Kr

  7. Development of two U.H.F. band resonators for application to CO2 laser electro-optical modulation

    International Nuclear Information System (INIS)

    Egan, M.G.; Blanc, P.; Sexton, M.C.

    1980-01-01

    The purpose of this report is to describe the design and testing of two U.H.F. band resonators destined for use in the linear electro-optical modulator of the CO 2 Laser Rapid Interferometer diagnostic at present under development for the WEGA Tokamak. The resonators take the form of a re-entrant coaxial line cavity and an interdigital line filter, both of which possess the regions of high electric field necessary to activate the linear electro-optical effect

  8. Compton harmonic resonances, stochastic instabilities, quasilinear diffusion, and collisionless damping with ultra-high intensity laser waves

    International Nuclear Information System (INIS)

    Rax, J.M.

    1992-04-01

    The dynamics of electrons in two-dimensional, linearly or circularly polarized, ultra-high intensity (above 10 18 W/cm 2 ) laser waves, is investigated. The Compton harmonic resonances are identified as the source of various stochastic instabilities. Both Arnold diffusion and resonance overlap are considered. The quasilinear kinetic equation, describing the evolution of the electron distribution function, is derived, and the associated collisionless damping coefficient is calculated. The implications of these new processes are considered and discussed

  9. Determination of iodine in oyster tissue by isotope dilution laser resonance ionization mass spectrometry

    International Nuclear Information System (INIS)

    Fassett, J.D.; Murphy, T.J.

    1990-01-01

    The technique of laser resonance ionization mass spectrometry has been combined with isotope dilution analysis to determine iodine in oyster tissue. The long-lived radioisotope, 129I, was used to spike the samples. Samples were equilibrated with the 129I, wet ashed under controlled conditions, and iodine separated by coprecipitation with silver chloride. The analyte was dried as silver ammonium iodide upon a tantalum filament from which iodine was thermally desorbed in the resonance ionization mass spectrometry instrument. A single-color, two-photon resonant plus one-photon ionization scheme was used to form positive iodine ions. Long-lived iodine signals were achieved from 100 ng of iodine. The precision of 127I/129I measurement has been evaluated by replicate determinations of the spike, the spike calibration samples, and the oyster tissue samples and was 1.0%. Measurement precision among samples was 1.9% for the spike calibration and 1.4% for the oyster tissue. The concentration of iodine determined in SRM 1566a, Oyster Tissue, was 4.44 micrograms/g with an estimate of the overall uncertainty for the analysis of +/- 0.12 microgram/g

  10. Tests of a grazing-incidence ring resonator free-electron laser

    International Nuclear Information System (INIS)

    Dowell, D.H.; Laucks, M.L.; Lowrey, A.R.; Adamski, J.L.; Pistoresi, D.J.; Shoffstall, D.R.; Bentz, M.P.; Burns, R.H.; Guha, J.; Sun, K.; Tomita, W.

    1991-01-01

    This paper reports on the Boeing free-electron laser (FEL) optical cavity that has been changed from a simple concentric cavity using two spherical mirrors to a larger grazing-incidence ring resonator. The new resonator consists of two mirror telescopes located at each end of the wiggler with a round-trip path length of approximately 133 m. Each telescope is a grazing-incidence hyperboloid followed by a normal-incidence paraboloid. Initial tests showed that poorly positioned ring focus and unreliable pointing alignment resulted in reduced and structured FEL output. (First lasing operation occurred on March 23 and 24, 1990.) Later efforts concentrated on improving the resonator alignment techniques and lowering the single-pass losses. FEL performance and reliability have significantly improved due to better ring alignment. The alignment procedure and recent lasing results are described. The effect the electron beam has on lasing is also discussed. Measurements are presented showing how FEL temporal output and wavelength are sensitive to electron beam energy variations

  11. IV-VI mid-IR tunable lasers and detectors with external resonant cavities

    Science.gov (United States)

    Zogg, H.; Rahim, M.; Khiar, A.; Fill, M.; Felder, F.; Quack, N.; Blunier, S.; Dual, J.

    2009-08-01

    Wavelength tunable emitters and detectors in the mid-IR wavelength region allow applications including thermal imaging and spectroscopy. Such devices may be realized using a resonant cavity. By mechanically changing the cavity length with MEMS mirror techniques, the wavelengths may be tuned over a considerable range. Vertical external cavity surface emitting lasers (VECSEL) may be applied for gas spectroscopy. Resonant cavity enhanced detectors (RCED) are sensitive at the cavity resonance only. They may be applied for low resolution spectroscopy, and, when arrays of such detectors are realized, as multicolor IR-FPA or IR-AFPA (IR-adaptive focal plane arrays). We review mid-infrared RCEDs and VECSELs using narrow gap IV-VI (lead chalcogenide) materials like PbTe and PbSe as the active medium. IV-VIs are fault tolerant and allow easy wavelength tuning. The VECSELs operate up to above room temperature and emit in the 4 - 5 μm range with a PbSe active layer. RCEDs with PbTe absorbing layers above 200 K operating temperature have higher sensitivities than the theoretical limit for a similar broad-band detector coupled with a passive tunable band-filter.

  12. Observation of double resonant laser induced transitions in the $v = n - l - 1 = 2$ metastable cascade of antiprotonic helium-4 atoms

    CERN Document Server

    Hayano, R S; Tamura, H; Torii, H A; Hori, Masaki; Maas, F E; Morita, N; Kumakura, M; Sugai, I; Hartmann, F J; Daniel, H; Von Egidy, T; Ketzer, B; Pohl, R; Horváth, D; Eades, John; Widmann, E; Yamazaki, T

    1997-01-01

    A new laser-induced resonant transition in the $v=n-l-1=2$ metastable cascade of antiprotonic $^4$He atoms has been found by using a double resonance technique. This was done by setting the first laser to the already known 470.724 nm resonance ($(n,l)=(37,34)\\rightarrow (36,33)$), while the $(38,35)\\rightarrow (37,34)$ transition was searched for with the second laser. The resonant transition was found at wavelength of 529.622$\\pm$0.003 nm, showing excellent agreement with a recent prediction of Korobov.

  13. Transportable high sensitivity small sample radiometric calorimeter

    International Nuclear Information System (INIS)

    Wetzel, J.R.; Biddle, R.S.; Cordova, B.S.; Sampson, T.E.; Dye, H.R.; McDow, J.G.

    1998-01-01

    A new small-sample, high-sensitivity transportable radiometric calorimeter, which can be operated in different modes, contains an electrical calibration method, and can be used to develop secondary standards, will be described in this presentation. The data taken from preliminary tests will be presented to indicate the precision and accuracy of the instrument. The calorimeter and temperature-controlled bath, at present, require only a 30-in. by 20-in. tabletop area. The calorimeter is operated from a laptop computer system using unique measurement module capable of monitoring all necessary calorimeter signals. The calorimeter can be operated in the normal calorimeter equilibration mode, as a comparison instrument, using twin chambers and an external electrical calibration method. The sample chamber is 0.75 in (1.9 cm) in diameter by 2.5 in. (6.35 cm) long. This size will accommodate most 238 Pu heat standards manufactured in the past. The power range runs from 0.001 W to <20 W. The high end is only limited by sample size

  14. Highly sensitive detection of a current ripple

    International Nuclear Information System (INIS)

    Aoki, Takashi; Gushiken, Tutomu; Nishikigouri, Kazutaka; Kumada, Masayuki.

    1996-01-01

    In the HIMAC, there are six thyristor-controlled power sources for driving two synchrotrons. These power sources are the three-output terminal power sources which are equipped with positive output, negative output and neutral point for the common mode countermeasures. As electromagnet circuits are connected to the three-output terminal power sources, those are three-line type. In the inside of the power source circuits controlled by thyristors, there is the oscillation peculiar to the power sources, and the variation of voltage induces current spikes. This time, in order to assess the results of the common mode countermeasures in the power source and electromagnet circuits, as one method of cross-check, it is considered that since electromagnet current flows being divided to the bridging resistance and the coil, if attention is paid to the current on bridging resistance side, the ripple components of common mode and normal mode can be detected with high sensitivity, and this was verified. The present state of heightening the performance of synchrotron power sources is explained. The cross-check of the method of assessing the performance of electromagnet power sources is reported. The method of measuring ripple current and the results of the measurement are reported. (K.I.)

  15. Development of high sensitivity radon detectors

    CERN Document Server

    Takeuchi, Y; Kajita, T; Tasaka, S; Hori, H; Nemoto, M; Okazawa, H

    1999-01-01

    High sensitivity detectors for radon in air and in water have been developed. We use electrostatic collection and a PIN photodiode for these detectors. Calibration systems have been also constructed to obtain collection factors. As a result of the calibration study, the absolute humidity dependence of the radon detector for air is clearly observed in the region less than about 1.6 g/m sup 3. The calibration factors of the radon detector for air are 2.2+-0.2 (counts/day)/(mBq/m sup 3) at 0.08 g/m sup 3 and 0.86+-0.06 (counts/day)/(mBq/m sup 3) at 11 g/m sup 3. The calibration factor of the radon detector for water is 3.6+-0.5 (counts/day)/(mBq/m sup 3). The background level of the radon detector for air is 2.4+-1.3 counts/day. As a result, one standard deviation excess of the signal above the background of the radon detector for air should be possible for 1.4 mBq/m sup 3 in a one-day measurement at 0.08 g/m sup 3.

  16. Time-resolved spectroscopy and fluorescence resonance energy transfer in the study of excimer laser damage of chromatin

    Energy Technology Data Exchange (ETDEWEB)

    Radu, L. [Department of Molecular Genetics and Radiobiology, Babes National Institute, Bucharest (Romania)], E-mail: lilianajradu@yahoo.fr; Mihailescu, I. [Department of Lasers, Laser, Plasma and Radiation Physics Institute, Bucharest (Romania); Radu, S. [Department of Computer Science, Polytechnics University, Bucharest (Romania); Gazdaru, D. [Department of Biophysics, Bucharest University (Romania)

    2007-09-21

    The analysis of chromatin damage produced by a 248 nm excimer laser radiation, for doses of 0.3-3 MJ/m{sup 2} was carried out by time-resolved spectroscopy and fluorescence resonance energy transfer (FRET). The chromatin was extracted from a normal and a tumoral tissue of Wistar rats. The decrease with laser dose of the relative contribution of the excited state lifetimes of ethidium bromide (EtBr) bounded to chromatin constitutes an evidence of the reduction of chromatin deoxyribonucleic acid (DNA) double-strand structure. FRET was performed from dansyl chloride to acridine orange, both coupled to chromatin. The increase of the average distance between these ligands, under the action of laser radiation, reflects a loosening of the chromatin structure. The radiosensitivity of tumor tissue chromatin is higher than that of a normal tissue. The determination of the chromatin structure modification in an excimer laser field can be of interest in laser therapy.

  17. Time-resolved spectroscopy and fluorescence resonance energy transfer in the study of excimer laser damage of chromatin

    International Nuclear Information System (INIS)

    Radu, L.; Mihailescu, I.; Radu, S.; Gazdaru, D.

    2007-01-01

    The analysis of chromatin damage produced by a 248 nm excimer laser radiation, for doses of 0.3-3 MJ/m 2 was carried out by time-resolved spectroscopy and fluorescence resonance energy transfer (FRET). The chromatin was extracted from a normal and a tumoral tissue of Wistar rats. The decrease with laser dose of the relative contribution of the excited state lifetimes of ethidium bromide (EtBr) bounded to chromatin constitutes an evidence of the reduction of chromatin deoxyribonucleic acid (DNA) double-strand structure. FRET was performed from dansyl chloride to acridine orange, both coupled to chromatin. The increase of the average distance between these ligands, under the action of laser radiation, reflects a loosening of the chromatin structure. The radiosensitivity of tumor tissue chromatin is higher than that of a normal tissue. The determination of the chromatin structure modification in an excimer laser field can be of interest in laser therapy

  18. The use of lasers as sources for Raman spectrometry, resonance Raman spectrometry, and light scattering

    International Nuclear Information System (INIS)

    Capitini, R.; Ceccaldi, M.; Leicknam, J.P.; Plus, R.

    1975-01-01

    The activity of the laboratory is principally centred on the determination of molecular structures and the study of molecular interactions in solution by infrared and Raman spectrometry. With the development of work on relatively large molecules, particularly biological molecules, it became necessary to complete information on the molecular weight and on the intra and intermolecular geometry and interactions of these bodies. In order to obtain these informations Rayleigh scattering and resonance Raman spectrometry were used. The advantages of using vibrational spectrometry, particularly Raman, in conjunction with the diffusion of light for these structural and molecular interaction studies is emphasized. It is shown that these two techniques could not have developed as they have done in the last few years without the use of lasers as light source [fr

  19. Resonator modes and mode dynamics for an external cavity-coupled laser array

    Science.gov (United States)

    Nair, Niketh; Bochove, Erik J.; Aceves, Alejandro B.; Zunoubi, Mohammad R.; Braiman, Yehuda

    2015-03-01

    Employing a Fox-Li approach, we derived the cold-cavity mode structure and a coupled mode theory for a phased array of N single-transverse-mode active waveguides with feedback from an external cavity. We applied the analysis to a system with arbitrary laser lengths, external cavity design and coupling strengths to the external cavity. The entire system was treated as a single resonator. The effect of the external cavity was modeled by a set of boundary conditions expressed by an N-by-N frequency-dependent matrix relation between incident and reflected fields at the interface with the external cavity. The coupled mode theory can be adapted to various types of gain media and internal and external cavity designs.

  20. Resonant laser power build-up in ALPS-A 'light shining through a wall' experiment

    International Nuclear Information System (INIS)

    Ehret, Klaus; Frede, Maik; Ghazaryan, Samvel; Hildebrandt, Matthias; Knabbe, Ernst-Axel; Kracht, Dietmar; Lindner, Axel; List, Jenny; Meier, Tobias; Meyer, Niels; Notz, Dieter; Redondo, Javier; Ringwald, Andreas; Wiedemann, Guenter; Willke, Benno

    2009-01-01

    The ALPS Collaboration runs a 'light shining through a wall' (LSW) experiment to search for photon oscillations into 'weakly interacting sub-eV particles' (WISPs) inside of a superconducting HERA dipole magnet at the site of DESY. In this paper we report on the first successful integration of a large-scale optical resonant cavity to boost the available power for WISP production in this type of experiments. The key elements are a frequency tunable narrow line-width continuous wave laser acting as the primary light source and an electronic feed-back control loop to stabilize the power build-up. We describe and characterize our apparatus and demonstrate the data analysis procedures on the basis of a brief exemplary run.

  1. Phase sensitive diffraction sensor for high sensitivity refractive index measurement

    Science.gov (United States)

    Kumawat, Nityanand; Varma, Manoj; Kumar, Sunil

    2018-02-01

    In this study a diffraction based sensor has been developed for bio molecular sensing applications and performing assays in real time. A diffraction grating fabricated on a glass substrate produced diffraction patterns both in transmission and reflection when illuminated by a laser diode. We used zeroth order I(0,0) as reference and first order I(0,1) as signal channel and conducted ratiometric measurements that reduced noise by more than 50 times. The ratiometric approach resulted in a very simple instrumentation with very high sensitivity. In the past, we have shown refractive index measurements both for bulk and surface adsorption using the diffractive self-referencing approach. In the current work we extend the same concept to higher diffraction orders. We have considered order I(0,1) and I(1,1) and performed ratiometric measurements I(0,1)/I(1,1) to eliminate the common mode fluctuations. Since orders I(0,1) and I(1,1) behaved opposite to each other, the resulting ratio signal amplitude increased more than twice compared to our previous results. As a proof of concept we used different salt concentrations in DI water. Increased signal amplitude and improved fluid injection system resulted in more than 4 times improvement in detection limit, giving limit of detection 1.3×10-7 refractive index unit (RIU) compared to our previous results. The improved refractive index sensitivity will help significantly for high sensitivity label free bio sensing application in a very cost-effective and simple experimental set-up.

  2. High sensitivity amplifier/discriminator for PWC's

    International Nuclear Information System (INIS)

    Hansen, S.

    1983-01-01

    The facility support group at Fermilab is designing and building a general purpose beam chamber for use in several locations at the laboratory. This pwc has 128 wires per plane spaced 1 mm apart. An initial production of 25 signal planes is anticipated. In proportional chambers, the size of the signal depends exponentially on the charge stored per unit of length along the anode wire. As the wire spacing decreases, the capacitance per unit length decreases, thereby requiring increased applied voltage to restore the necessary charge per unit length. In practical terms, this phenomenon is responsible for difficulties in constructing chambers with less than 2 mm wire spacing. 1 mm chambers, therefore, are frequently operated very near to their breakdown point and/or a high gain gas containing organic compounds such as magic gas is used. This argon/iso-butane mixture has three drawbacks: it is explosive when exposed to the air, it leaves a residue on the wires after extended use and is costly. An amplifier with higher sensitivity would reduce the problems associated with operating chambers with small wire spacings and allow them to be run a safe margin below their breakdown voltage even with an inorganic gas mixture such as argon/CO2, this eliminating the need to use magic gas. Described here is a low cost amplifier with a usable threshold of less than 0.5 μA. Data on the performance of this amplifier/discriminator in operation on a prototype beam chamber are given. This data shows the advantages of the high sensitivity of this design

  3. Computational study of plasma-assisted photoacoustic response from gold nanoparticles irradiated by off-resonance ultrafast laser

    International Nuclear Information System (INIS)

    Hatef, Ali; Darvish, Behafarid; Sajjadi, Amir Yousef

    2017-01-01

    The gold nanoparticles (AuNPs) are capable of enhancing the incident laser field in the form of scattered near field for even an off-resonance irradiation where the incident laser wavelength is far away from the localized surface plasmon resonance (LSPR). If the intensity of the pulse laser is large enough, this capability can be employed to generate a highly localized free electron (plasma) in the vicinity of the particles. The generated plasma can absorb more energy during the pulse, and this energy deposition can be considered as an energy source for structural mechanics calculations in the surrounding media to generate a photoacoustic (PA) signal. To show this, in this paper, we model plasma-mediated PA pressure wave propagation from a 100-nm AuNPs and the surrounding media irradiated by an ultrashort pulse laser. In this model, the AuNP is immersed in water and the laser pulse width is ranging from 70 fs to 2 ps at the wavelength of 800 nm (off-resonance). Our results qualitatively show the substantial impact of the energy deposition in plasma on the PA signal through boosting the pressure amplitudes up to ∼1000 times compared to the conventional approach.

  4. Computational study of plasma-assisted photoacoustic response from gold nanoparticles irradiated by off-resonance ultrafast laser

    Energy Technology Data Exchange (ETDEWEB)

    Hatef, Ali, E-mail: alih@nipissingu.ca; Darvish, Behafarid [Nipissing University, Nipissing Computational Physics Laboratory (NCPL), Department of Computer Science and Mathematics (Canada); Sajjadi, Amir Yousef [Massachusetts General Hospital, Cutaneous Biology Research Center (United States)

    2017-02-15

    The gold nanoparticles (AuNPs) are capable of enhancing the incident laser field in the form of scattered near field for even an off-resonance irradiation where the incident laser wavelength is far away from the localized surface plasmon resonance (LSPR). If the intensity of the pulse laser is large enough, this capability can be employed to generate a highly localized free electron (plasma) in the vicinity of the particles. The generated plasma can absorb more energy during the pulse, and this energy deposition can be considered as an energy source for structural mechanics calculations in the surrounding media to generate a photoacoustic (PA) signal. To show this, in this paper, we model plasma-mediated PA pressure wave propagation from a 100-nm AuNPs and the surrounding media irradiated by an ultrashort pulse laser. In this model, the AuNP is immersed in water and the laser pulse width is ranging from 70 fs to 2 ps at the wavelength of 800 nm (off-resonance). Our results qualitatively show the substantial impact of the energy deposition in plasma on the PA signal through boosting the pressure amplitudes up to ∼1000 times compared to the conventional approach.

  5. Resonant infrared laser deposition of polymer-nanocomposite materials for optoelectronic applications

    Science.gov (United States)

    Park, Hee K.; Schriver, Kenneth E.; Haglund, Richard F.

    2011-11-01

    Polymers find a number of potentially useful applications in optoelectronic devices. These include both active layers, such as light-emitting polymers and hole-transport layers, and passive layers, such as polymer barrier coatings and light-management films. This paper reports the experimental results for polymer films deposited by resonant infrared matrix-assisted pulsed laser evaporation (RIR-MAPLE) and resonant infrared pulsed laser deposition (RIR-PLD) for commercial optoelectronic device applications. In particular, light-management films, such as anti-reflection coatings, require refractive-index engineering of a material. However, refractive indices of polymers fall within a relatively narrow range, leading to major efforts to develop both low- and high-refractive-index polymers. Polymer nanocomposites can expand the range of refractive indices by incorporating low- or high-refractive-index nanoscale materials. RIR-MAPLE is an excellent technique for depositing polymer-nanocomposite films in multilayer structures, which are essential to light-management coatings. In this paper, we report our efforts to engineer the refractive index of a barrier polymer by combining RIR-MAPLE of nanomaterials (for example, high refractive-index TiO2 nanoparticles) and RIR-PLD of host polymer. In addition, we report on the properties of organic and polymer films deposited by RIR-MAPLE and/or RIR-PLD, such as Alq3 [tris(8-hydroxyquinoline) aluminum] and PEDOT:PSS [poly(3,4-ethylenedioxythiophene): poly(styrenesulfonate)]. Finally, the challenges and potential for commercializing RIR-MAPLE/PLD, such as industrial scale-up issues, are discussed.

  6. Laser-polarized xenon-129 magnetic resonance spectroscopy and imaging. The development of a method for in vivo perfusion measurement

    Science.gov (United States)

    Rosen, Matthew Scot

    2001-07-01

    This thesis presents in vivo nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) studies with laser-polarized 129Xe delivered to living rats by inhalation and transported to tissue via blood flow. The results presented herein include the observation, assignment, and dynamic measurement of 129Xe resonances in the brain and body, the first one- and two-dimensional chemical-shift-resolved images of 129Xe in blood, tissue, and gas in the thorax, and the first images of 129Xe in brain tissue. These results establish that laser-polarized 129Xe can be used as a magnetic resonance tracer in vivo. NMR resonances at 0, 191, 198, and 209 ppm relative to the 129 Xe gas resonance are observed in the rat thorax and assigned to 129Xe in gas, fat, tissue, and blood respectively. Resonances at 189, 192, 195, 198, and 209 ppm are observed in the brain, and the 195 and 209 ppm resonances are assigned to 129Xe in grey matter, and blood, respectively. The design and construction of a laser-polarized 129Xe production and delivery system is described. This system produces liter-volumes of laser- polarized 129Xe by spin-exchange optical- pumping. It represented an order of magnitude increase over previously reported production volumes of polarized 129Xe. At approximately 3-7% polarization, 157 cc-atm of xenon is produced and stored as ice every 5 minutes. This reliable, effective, and simple production method for large volumes of 129Xe can be applied to other areas of research involving the use of laser-polarized noble gases. A model of the in vivo transport of laser polarized 129Xe to tissue under realistic experimental NMR conditions is described. Appropriate control of the NMR parameters is shown to allow tissue perfasion and 129Xe tissue T1 to be extracted from measurement of the steady-state 129Xe tissue signal. In vivo rodent 129Xe NMR results are used to estimate the signal-to-noise ratio of this technique, and an inhaled 30% xenon/70% O2 mixture polarized to 5

  7. Selective Two-Photon Absorptive Resonance Femtosecond-Laser Electronic-Excitation Tagging (STARFLEET) Velocimetry in Flow and Combustion Diagnostics

    Science.gov (United States)

    Jiang, Naibo; Halls, Benjamin R.; Stauffer, Hans U.; Roy, Sukesh; Danehy, Paul M.; Gord, James R.

    2016-01-01

    Selective Two-Photon Absorptive Resonance Femtosecond-Laser Electronic-Excitation Tagging (STARFLEET), a non-seeded ultrafast-laser-based velocimetry technique, is demonstrated in reactive and non-reactive flows. STARFLEET is pumped via a two-photon resonance in N2 using 202.25-nm 100-fs light. STARFLEET greatly reduces the per-pulse energy required (30 µJ/pulse) to generate the signature FLEET emission compared to the conventional FLEET technique (1.1 mJ/pulse). This reduction in laser energy results in less energy deposited in the flow, which allows for reduced flow perturbations (reactive and non-reactive), increased thermometric accuracy, and less severe damage to materials. Velocity measurements conducted in a free jet of N2 and in a premixed flame show good agreement with theoretical velocities and further demonstrate the significantly less-intrusive nature of STARFLEET.

  8. Resonantly cladding-pumped Yb-free Er-doped LMA fiber laser with record high power and efficiency.

    Science.gov (United States)

    Zhang, Jun; Fromzel, Viktor; Dubinskii, Mark

    2011-03-14

    We report the results of our power scaling experiments with resonantly cladding-pumped Er-doped eye-safe large mode area (LMA) fiber laser. While using commercial off-the-shelf LMA fiber we achieved over 88 W of continuous-wave (CW) single transverse mode power at ~1590 nm while pumping at 1532.5 nm. Maximum observed optical-to-optical efficiency was 69%. This result presents, to the best of our knowledge, the highest power reported from resonantly-pumped Yb-free Er-doped LMA fiber laser, as well as the highest efficiency ever reported for any cladding-pumped Er-doped laser, either Yb-co-doped or Yb-free.

  9. Real time detection of antibody-antigen interaction using a laser scanning confocal imaging-surface plasmon resonance system

    International Nuclear Information System (INIS)

    Zhang Hong-Yan; Yang Li-Quan; Ning Ting-Yin; Liu Wei-Min; Sun Jia-Yu; Wang Peng-Fei; Meng Lan; Nie Jia-Cai

    2012-01-01

    A laser scanning confocal imaging-surface plasmon resonance (LSCI-SPR) instrument integrated with a wavelength-dependent surface plasmon resonance (SPR) sensor and a laser scanning confocal microscopy (LSCM) is built to detect the bonding process of human IgG and fluorescent-labeled affinity purified antibodies in real time. The shifts of resonant wavelength at different reaction time stages are obtained by SPR, corresponding well with the changes of the fluorescence intensity collected by using LSCM. The instrument shows the merits of the combination and complementation of the SPR and LSCM, with such advantages as quantificational analysis, high spatial resolution and real time monitor, which are of great importance for practical applications in biosensor and life science. (general)

  10. Hot-cavity studies for the Resonance Ionization Laser Ion Source

    International Nuclear Information System (INIS)

    Henares, J.L.; Lecesne, N.; Hijazi, L.; Bastin, B.; Kron, T.; Lassen, J.; Le Blanc, F.; Leroy, R.; Osmond, B.; Raeder, S.; Schneider, F.; Wendt, K.

    2016-01-01

    The Resonance Ionization Laser Ion Source (RILIS) has emerged as an important technique in many Radioactive Ion Beam (RIB) facilities for its reliability, and ability to ionize target elements efficiently and element selectively. GISELE is an off-line RILIS test bench to study the implementation of an on-line laser ion source at the GANIL separator facility. The aim of this project is to determine the best technical solution which combines high selectivity and ionization efficiency with small ion beam emittance and stable long term operation. The ion source geometry was tested in several configurations in order to find a solution with optimal ionization efficiency and beam emittance. Furthermore, a low work function material was tested to reduce the contaminants and molecular sidebands generated inside the ion source. First results with ZrC ionizer tubes will be presented. Furthermore, a method to measure the energy distribution of the ion beam as a function of the time of flight will be discussed.

  11. Contactless respiratory monitoring system for magnetic resonance imaging applications using a laser range sensor

    Directory of Open Access Journals (Sweden)

    Krug Johannes W.

    2016-09-01

    Full Text Available During a magnetic resonance imaging (MRI exam, a respiratory signal can be required for different purposes, e.g. for patient monitoring, motion compensation or for research studies such as in functional MRI. In addition, respiratory information can be used as a biofeedback for the patient in order to control breath holds or shallow breathing. To reduce patient preparation time or distortions of the MR imaging system, we propose the use of a contactless approach for gathering information about the respiratory activity. An experimental setup based on a commercially available laser range sensor was used to detect respiratory induced motion of the chest or abdomen. This setup was tested using a motion phantom and different human subjects in an MRI scanner. A nasal airflow sensor served as a reference. For both, the phantom as well as the different human subjects, the motion frequency was precisely measured. These results show that a low cost, contactless, laser-based approach can be used to obtain information about the respiratory motion during an MRI exam.

  12. A low cost surface plasmon resonance biosensor using a laser line generator

    Science.gov (United States)

    Chen, Ruipeng; Wang, Manping; Wang, Shun; Liang, Hao; Hu, Xinran; Sun, Xiaohui; Zhu, Juanhua; Ma, Liuzheng; Jiang, Min; Hu, Jiandong; Li, Jianwei

    2015-08-01

    Due to the instrument designed by using a common surface plasmon resonance biosensor is extremely expensive, we established a portable and cost-effective surface plasmon resonance biosensing system. It is mainly composed of laser line generator, P-polarizer, customized prism, microfluidic cell, and line Charge Coupled Device (CCD) array. Microprocessor PIC24FJ128GA006 with embedded A/D converter, communication interface circuit and photoelectric signal amplifier circuit are used to obtain the weak signals from the biosensing system. Moreover, the line CCD module is checked and optimized on the number of pixels, pixels dimension, output amplifier and the timing diagram. The micro-flow cell is made of stainless steel with a high thermal conductivity, and the microprocessor based Proportional-Integral-Derivative (PID) temperature-controlled algorithm was designed to keep the constant temperature (25 °C) of the sample solutions. Correspondingly, the data algorithms designed especially to this biosensing system including amplitude-limiting filtering algorithm, data normalization and curve plotting were programmed efficiently. To validate the performance of the biosensor, ethanol solution samples at the concentrations of 5%, 7.5%, 10%, 12.5% and 15% in volumetric fractions were used, respectively. The fitting equation ΔRU = - 752987.265 + 570237.348 × RI with the R-Square of 0.97344 was established by delta response units (ΔRUs) to refractive indexes (RI). The maximum relative standard deviation (RSD) of 4.8% was obtained.

  13. Even-parity resonances with synchrotron radiation from Laser Excited Lithium at 1s^22p State

    Science.gov (United States)

    Huang, Ming-Tie; Wehlitz, Ralf

    2010-03-01

    Correlated many-body dynamics is still one of the unsolved fundamental problems in physics. Such correlation effects can be most clearly studied in processes involving single atoms for their simplicity.Lithium, being the simplest open shell atom, has been under a lot of study. Most of the studies focused on ground state lithium. However, only odd parity resonances can be populated through single photon (synchrotron radiation) absorption from ground state lithium (1s^22s). Lithium atoms, after being laser excited to the 1s^22p state, allow the study of even parity resonances. We have measured some of the even parity resonances of lithium for resonant energies below 64 eV. A single-mode diode laser is used to excite lithium from 1s^22s ground state to 1s^22p (^2P3/2) state. Photoions resulting from the interaction between the excited lithium and synchrotron radiation were analyzed and collected by an ion time-of-flight (TOF) spectrometer with a Z- stack channel plate detector. The Li^+ ion yield was recorded while scanning the undulator along with the monochromator. The energy scans have been analyzed regarding resonance energies and parameters of the Fano profiles. Our results for the observed resonances will be presented.

  14. Resonance

    DEFF Research Database (Denmark)

    Petersen, Nils Holger

    2014-01-01

    A chapter in a book about terminology within the field of medievalism: the chapter discusses the resonance of medieval music and ritual in modern (classical) music culture and liturgical practice.......A chapter in a book about terminology within the field of medievalism: the chapter discusses the resonance of medieval music and ritual in modern (classical) music culture and liturgical practice....

  15. Blue diode laser versus traditional infrared diode laser and quantic molecular resonance scalpel: clinical and histological findings after excisional biopsy of benign oral lesions

    Science.gov (United States)

    Gobbo, Margherita; Bussani, Rossana; Perinetti, Giuseppe; Rupel, Katia; Bevilaqua, Lorenzo; Ottaviani, Giulia; Biasotto, Matteo

    2017-12-01

    This study aims to compare the use of the innovative blue diode laser (BLUE group) with two traditional surgical techniques: the infrared diode laser (IR group) and the quantic molecular resonance scalpel (QMR group) in the excision of benign oral lesions. Ninety-three patients underwent surgical excision of a benign oral lesion and were followed up for 30 days for pain (0 to 10 visual analogue scale), bleeding, and painkillers' assumption (yes/no). A blind pathologist evaluated the thermal damage along the cutting margin. Although referred pain was lowest in the BLUE group from day 7 on (plaser minimizes risk of bleeding with limited thermal damage.

  16. High-power Nd:YAG lasers using stable-unstable resonators

    CERN Document Server

    Mudge, D; Ottaway, D J; Veitch, P J; Munch, J P; Hamilton, M W

    2002-01-01

    The development of a power-scalable diode-laser-pumped continuous-wave Nd:YAG laser for advanced long-baseline interferometric detectors of gravitational waves is described. The laser employs a chain of injection-locked slave lasers to yield an efficient, frequency-stable, diffraction-limited laser beam.

  17. Three-Rod Resonator for Krypton Lamp Pumped 1.8 kW Continuous-Wave Nd:YAG Laser

    Institute of Scientific and Technical Information of China (English)

    LI Qiang; FANG Ming-Xing; WANG Zhi-Yong; YU Zhen-Sheng; LEI Hong; GUO Jiang; LI Gang; ZUO Tie-Chuan

    2004-01-01

    @@ A three-rod series resonator cw Nd:YAG laser suitable for the industrial applications is presented. The symmetrical resonator laser has been developed and is rated at 1820-W output power with beam parameter product 24 mm.mrad. By utilizing the symmetrical resonator design, the characteristic of beam with multi-rod is not obviously decreased compared with that of a single one. The system total electro-optics efficiency of lamp pumped YAG crystal is as high as 4.0%. The main factors, which affect output power and beam quality of high power solid-state laser module, are theoretically analysed.

  18. Laser Raman and resonance Raman spectroscopies of natural semiconductor mineral cinnabar, α-HgS, from various mines

    International Nuclear Information System (INIS)

    Gotoshia, Sergo V; Gotoshia, Lamara V

    2008-01-01

    Natural minerals α-HgS from various mines have been studied by laser Raman spectroscopy and resonance Raman spectroscopy. The crystals differ from each other in the content of selenium impurity, included in samples from some mines. Based on the Raman spectra and the factor-group analysis the classification of the first order phonons and then the comparison of the results with the results from other works were carried out. The Raman spectra analysis of minerals from various mines show the selenium impurity gap vibration at 203 cm -1 and 226 cm -1 frequencies, respectively. On the basis of statistical measurements of the Raman spectra one can conclude that impurity frequencies of α-HgS may be generally used for the identification of the mine. Resonance Raman scattering for pure minerals has been studied by a dye laser. Phonon resonance in the indirect semiconductor α-HgS is found to be far more intense than the indirect resonance detected until now in various semiconductors in the proximity of the first indirect band E g , for instance, in GaP. In our opinion, this may be conditioned by cinnabar band structure peculiarities. Low resonance has also been fixed in 'dirty' minerals at the spectral band frequency of 203 cm -1 characterizing gap vibration of isomorphic impurity Se in cinnabar

  19. Determination of organic compounds in nano-particles by laser breakdown and resonant ionization time-of-flight mass spectrometry

    International Nuclear Information System (INIS)

    Deguchi, Yoshihiro; Tanaka, Nobuyuki

    2005-01-01

    Laser breakdown and resonance ionization time-of-flight mass spectrometry (TOFMS) with a differential mobility analyzer (DMA) was developed and applied to detect compositions and organic substances in nano-particles. The laser breakdown TOFMS method is capable of reaching pptv sensitivity, which is generally much better than the normal LIBS techniques. The system was demonstrated to successfully detect signals in the mass range of 1 to 300 amu for 60 and 140 nm particles in diesel engine exhaust. The detected signals showed that the nano-particles contained both aromatic and chain hydrocarbons

  20. Characteristics of laser irradiated Hg sub 0 ,835 Cd sub 0 ,165 Te analysed by resonant Raman spectroscopy

    International Nuclear Information System (INIS)

    Scepanovic, M.; Jevtic, M.

    1998-01-01

    The characteristics of Hg sub 0 ,835 Cd sub 0 ,165 Te sample irradiated by a nanosecond Nd: YAG laser pulse are investigated using a resonant Raman spectroscopy. The pulse energy density of 100 mJ/cm sup 2 is close to the energy threshold of material melting under the irradiated conditions. The presented Raman spectra of the unirradiated and irradiated sample parts point out that the laser irradiation induced a little concentration change in the surface sample layers without the essential structural changes (author)

  1. Lithographic wavelength control of an external cavity laser with a silicon photonic crystal cavity-based resonant reflector.

    Science.gov (United States)

    Liles, Alexandros A; Debnath, Kapil; O'Faolain, Liam

    2016-03-01

    We report the experimental demonstration of a new design for external cavity hybrid lasers consisting of a III-V semiconductor optical amplifier (SOA) with fiber reflector and a photonic crystal (PhC)-based resonant reflector on SOI. The silicon reflector is composed of an SU8 polymer bus waveguide vertically coupled to a PhC cavity and provides a wavelength-selective optical feedback to the laser cavity. This device exhibits milliwatt-level output power and side-mode suppression ratios of more than 25 dB.

  2. High-precision hyperfine structure measurement in slow atomic ion beams by collinear laser-rf double resonance

    International Nuclear Information System (INIS)

    Amarjit Sen; Childs, W.J.; Goodman, L.S.

    1987-01-01

    A new collinear laser-ion beam apparatus for slow ions (1 to 1.5 keV) has been built for measuring the hyperfine structure of metastable levels of ions with laser-rf double resonance technique. Narrow linewidths of ∼60 kHz (FWHM) have been observed for the first time in such systems. As a first application the hyperfine structure of the 4f 7 ( 8 S 0 )5d 9 D/sub J/ 0 metastable levels of /sup 151,153/Eu + has been measured with high precision. 10 refs., 8 figs

  3. Application of quantum-dot multi-wavelength lasers and silicon photonic ring resonators to data-center optical interconnects

    Science.gov (United States)

    Beckett, Douglas J. S.; Hickey, Ryan; Logan, Dylan F.; Knights, Andrew P.; Chen, Rong; Cao, Bin; Wheeldon, Jeffery F.

    2018-02-01

    Quantum dot comb sources integrated with silicon photonic ring-resonator filters and modulators enable the realization of optical sub-components and modules for both inter- and intra-data-center applications. Low-noise, multi-wavelength, single-chip, laser sources, PAM4 modulation and direct detection allow a practical, scalable, architecture for applications beyond 400 Gb/s. Multi-wavelength, single-chip light sources are essential for reducing power dissipation, space and cost, while silicon photonic ring resonators offer high-performance with space and power efficiency.

  4. Bloch surface wave structures for high sensitivity detection and compact waveguiding

    Science.gov (United States)

    Khan, Muhammad Umar; Corbett, Brian

    2016-01-01

    Resonant propagating waves created on the surface of a dielectric multilayer stack, called Bloch surface waves (BSW), can be designed for high sensitivity monitoring of the adjacent refractive index as an alternative platform to the metal-based surface plasmon resonance (SPR) sensing. The resonant wavelength and polarization can be designed by engineering of the dielectric layers unlike the fixed resonance of SPR, while the wide bandwidth low loss of dielectrics permits sharper resonances, longer propagation lengths and thus their use in waveguiding devices. The transparency of the dielectrics allows the excitation and monitoring of surface-bound fluorescent molecules. We review the recent developments in this technology. We show the advantages that can be obtained by using high index contrast layered structures. Operating at 1550 nm wavelengths will allow the BSW sensors to be implemented in the silicon photonics platform where active waveguiding can be used in the realization of compact planar integrated circuits for multi-parameter sensing.

  5. Continuous-wave generation and tunability of eye-safe resonantly diode-pumped Er:YAG laser

    Science.gov (United States)

    Němec, Michal; Indra, Lukás.; Šulc, Jan; Jelínková, Helena

    2016-03-01

    Laser sources generating radiation in the spectral range from 1.5 to 1.7 μm are very attractive for many applications such as satellite communication, range finding, spectroscopy, and atmospheric sensing. The goal of our research was an investigation of continuous-wave generation and wavelength tuning possibility of diode pumped eye-safe Er:YAG laser emitting radiation around 1645 nm. We used two 0.5 at. % doped Er:YAG active media with lengths of 10 mm and 25 mm (diameter 5 mm). As a pumping source, a fibre-coupled 1452 nm laser-diode was utilized, which giving possibility of the in-band pumping with a small quantum defect and low thermal stress of the active bulk laser material. The 150 mm long resonator was formed by a pump mirror (HT @ 1450 nm, HR @ 1610 - 1660 nm) and output coupler with 96 % reflectivity at 1610 - 1660 nm. For continuous-wave generation, the maximal output powers were 0.7 W and 1 W for 10 mm and 25 mm long laser crystals, respectively. The corresponding slope efficiencies with respect to absorbed pump power for these Er:YAG lasers were 26.5 % and 37.8 %, respectively. The beam spatial structure was close to the fundamental Gaussian mode. A wavelength tunability was realized by a birefringent plate and four local spectral maxima at 1616, 1633, 1645, and 1657 nm were reached. The output characteristics of the designed and realized resonantly diode-pumped eye-safe Er:YAG laser show that this compact system has a potential for usage mainly in spectroscopic fields.

  6. Demonstration of resonant photopumping of Mo VII by Mo XII for a VUV laser near 600 Angstrom

    International Nuclear Information System (INIS)

    Ilcisin, K.J.; Aumayr, F.; Schwob, J.L.; Suckewer, S.

    1993-09-01

    We present data of experiments on the resonant photopumping of Mo VII by Mo XII as a method of generating a coherent VUV source near 600 angstrom. The experiment is based on a scheme proposed by Feldman and Reader in which the 4p 6 -- 4p 5 6s transition in Mo VII in resonantly photopumped by the 5s 2 S 1/2 -- 4p 2 P 1/2 transition in Mo XII. Results of the laser produced plasma experiments show the successful enhancement of the population of the Mo VII 4p 5 6s upper lasing level when pumped by an adjacent Mo VII plasma. No enhancement was seen in a control experiment where the Mo VII plasma was pumped by a Zr X plasma. Improvements of the intensity of the Mo XII pump source, achieved using an additional pump laser, lead to the generation of a population inversion for the VUV transition

  7. Beta-decay measurements of neutron-rich thallium, lead, and bismuth by means of resonant laser ionisation

    Science.gov (United States)

    Franchoo, S.; de Witte, H.; Andreyev, A. N.; Cederka¨Ll, J.; Dean, S.; de Smet, A.; Eeckhaudt, S.; Fedorov, D. V.; Fedosseev, V. N.; G´Rska, M.; Huber, G.; Huyse, M.; Janas, Z.; Ko¨Ster, U.; Kurcewicz, W.; Kurpeta, J.; Mayer, P.; Płchocki, A.; van de Vel, K.; van Duppen, P.; Weissman, L.; Isolde Collaboration

    2004-04-01

    Neutron-rich thallium, lead, and bismuth isotopes were investigated at the ISOLDE facility. After mass separation and resonant laser ionisation of the produced activity, new spectroscopic data were obtained for 215,218Bi and 215Pb. An attempt to reach heavy thallium had to be abandoned because of a strong francium component in the beam that gave rise to a neutron background through (α,n) reactions on the aluminium walls of the experimental chamber.

  8. Study of the ionization of sodium vapor in the presence of resonant laser radiation

    International Nuclear Information System (INIS)

    Carre, B.

    1986-06-01

    Ionization of a diffuse sodium jet, excited by laser radiation (D2 resonance), either continuous or pulsed, is studied by electron spectroscopy. Results show: associative ionization (AI) in the collision of two Na(3p) excited atoms; occupancy of highly excited nl states in energy association collisions of two Na(3p) followed by Penning collisional ionization (CI) in the system Na(nl) + Na(3p); heating of electrons by 1, 2, or 3 superelastic collisions with Na(3p). For both the excitation cases (continuous or pulsed source) analysis of experiment results leads to a description of the whole of the ionized medium, characterized as being low density and the site of the ambipolar diffusion of charged particles. A highly simplified model describes the kinetic and electrokinetic equilibrium (continuous case) in which the different populations of distinct nonthermalized energy (low energy primary electrons, hot electrons) play specific roles. The cross sections associated with AI and CI are estimated from experiment results using the model [fr

  9. Resonant Infrared Matrix-Assisted Pulsed Laser Evaporation Of Inorganic Nanoparticles And Organic/Inorganic Hybrid Nanocomposites

    Science.gov (United States)

    Pate, Ryan; Lantz, Kevin R.; Dhawan, Anuj; Vo-Dinh, Tuan; Stiff-Roberts, Adrienne D.

    2010-10-01

    In this research, resonant infrared matrix-assisted pulsed laser evaporation (RIR-MAPLE) has been used to deposit different classes of inorganic nanoparticles, including bare, un-encapsulated ZnO and Au nanoparticles, as well as ligand-encapsulated CdSe colloidal quantum dots (CQDs). RIR-MAPLE has been used for thin-film deposition of different organic/inorganic hybrid nanocomposites using some of these inorganic nanoparticles, including CdSe CQD-poly[2-methoxy-5-(2'-ethylhexyloxy)-1,4-(1-cyanovinylene)phenylene] (MEH-CN-PPV) nanocomposites and Au nanoparticle-poly(methyl methacrylate) (PMMA) nanocomposites. The unique contribution of this research is that a technique is demonstrated for the deposition of organic-based thin-films requiring solvents with bond energies that do not have to be resonant with the laser energy. By creating an emulsion of solvent and ice in the target, RIR-MAPLE using a 2.94 μm laser can deposit most material systems because the hydroxyl bonds in the ice component of the emulsion matrix are strongly resonant with the 2.94 μm laser. In this way, the types of materials that can be deposited using RIR-MAPLE has been significantly expanded. Furthermore, materials with different solvent bond energies can be co-deposited without concern for material degradation and without the need to specifically tune the laser energy to each material solvent bond energy, thereby facilitating the realization of organic/inorganic hybrid nanocomposite thin-films. In addition to the structural characterization of the inorganic nanoparticle and hybrid nanocomposite thin-films deposited using this RIR-MAPLE technique, optical characterization is presented to demonstrate the potential of such films for optoelectronic device applications.

  10. Resonant Infrared Matrix-Assisted Pulsed Laser Evaporation Of Inorganic Nanoparticles And Organic/Inorganic Hybrid Nanocomposites

    International Nuclear Information System (INIS)

    Pate, Ryan; Lantz, Kevin R.; Stiff-Roberts, Adrienne D.; Dhawan, Anuj; Vo-Dinh, Tuan

    2010-01-01

    In this research, resonant infrared matrix-assisted pulsed laser evaporation (RIR-MAPLE) has been used to deposit different classes of inorganic nanoparticles, including bare, un-encapsulated ZnO and Au nanoparticles, as well as ligand-encapsulated CdSe colloidal quantum dots (CQDs). RIR-MAPLE has been used for thin-film deposition of different organic/inorganic hybrid nanocomposites using some of these inorganic nanoparticles, including CdSe CQD-poly[2-methoxy-5-(2'-ethylhexyloxy )-1,4-(1-cyanovinylene)phenylene](MEH-CN-PPV) nanocomposites and Au nanoparticle-poly(methyl methacrylate)(PMMA) nanocomposites. The unique contribution of this research is that a technique is demonstrated for the deposition of organic-based thin-films requiring solvents with bond energies that do not have to be resonant with the laser energy. By creating an emulsion of solvent and ice in the target, RIR-MAPLE using a 2.94 μm laser can deposit most material systems because the hydroxyl bonds in the ice component of the emulsion matrix are strongly resonant with the 2.94 μm laser. In this way, the types of materials that can be deposited using RIR-MAPLE has been significantly expanded. Furthermore, materials with different solvent bond energies can be co-deposited without concern for material degradation and without the need to specifically tune the laser energy to each material solvent bond energy, thereby facilitating the realization of organic/inorganic hybrid nanocomposite thin-films. In addition to the structural characterization of the inorganic nanoparticle and hybrid nanocomposite thin-films deposited using this RIR-MAPLE technique, optical characterization is presented to demonstrate the potential of such films for optoelectronic device applications.

  11. Resonance Raman scattering of β-carotene solution excited by visible laser beams into second singlet state.

    Science.gov (United States)

    Lu, Luyao; Shi, Lingyan; Secor, Jeff; Alfano, Robert

    2018-02-01

    This study aimed to use self-absorption correction to determine the Raman enhancement of β-carotene. The Raman spectra of β-carotene solutions were measured using 488nm, 514nm, 532nm and 633nm laser beams, which exhibited significant resonance Raman (RR) enhancement when the laser energy approaches the electronic transition energy from S 0 to S 2 state. The Raman intensity and the actual resonance Raman gain without self-absorption from S 2 state by β-carotene were also obtained to evaluate the effect of self-absorption on RR scattering. Moreover, we observed the Raman intensity strength followed the absorption spectra. Our study found that, although 488nm and 514nm pumps seemed better for stronger RR enhancement, 532nm would be the optimum Raman pump laser with moderate RR enhancement due to reduced fluorescence and self-absorption. The 532nm excitation will be helpful for applying resonance Raman spectroscopy to investigate biological molecules in tissues. Copyright © 2017 Elsevier B.V. All rights reserved.

  12. Nanowire-templated microelectrodes for high-sensitivity pH detection

    DEFF Research Database (Denmark)

    Antohe, V.A.; Radu, Adrian; Mátéfi-Tempfli, Mária

    2009-01-01

    A highly sensitive pH capacitive sensor has been designed by confined growth of vertically aligned nanowire arrays on interdigited microelectrodes. The active surface of the device has been functionalized with an electrochemical pH transducer (polyaniline). We easily tune the device features...... by combining lithographic techniques with electrochemical synthesis. The reported electrical LC resonance measurements show considerable sensitivity enhancement compared to conventional capacitive pH sensors realized with microfabricated interdigited electrodes. The sensitivity can be easily improved...

  13. Resonances

    DEFF Research Database (Denmark)

    an impetus or drive to that account: change, innovation, rupture, or discontinuity. Resonances: Historical Essays on Continuity and Change explores the historiographical question of the modes of interrelation between these motifs in historical narratives. The essays in the collection attempt to realize...

  14. Resonantly-enhanced, four-photon ionization of krypton at laser intensities exceeding 1013 W/cm2

    International Nuclear Information System (INIS)

    Perry, M.D.; Landen, O.L.; Campbell, E.M.

    1987-12-01

    The yield of singly- and multiply- charged ions of krypton and xenon is presented as a function of laser intensity and frequency. The measurements were performed using the second harmonic output of a well-characterized, tunable picosecond dye laser in the range 285 to 310 nm at laser intensities from 1 x 10 12 to 10 14 W/cm 2 . Enhancement of the Kr + yield by two orders of magnitude by three-photon resonant, four-photon ionization is observed in the vicinity of the 4d'[5/2] 3 and the 4d[3/2] 1 intermediate states. A model incorporating line shifts and widths scaling linearly with intensity is in good agreement with the experimental results

  15. Redox reactions of cytochrome c in isolated mitochondria exposed to blue or red lasers using resonance Raman spectroscopy

    Science.gov (United States)

    Denton, Michael L.; Gonzalez, Cherry C.; Noojin, Gary D.; Yakovlev, Vladislav V.

    2018-02-01

    Resonance Raman spectroscopy of cytochrome c was used to follow reduction/oxidation (redox) states of isolated mitochondria in response to blue or red laser exposure. Mitochondria were isolated from hTERT-RPE1 cells and were kept in a buffer formulation known to be conducive to electron transport chain (ETC) activity. Using either pyruvate or succinate as substrates for ETC, we found differences in the redox responses of cytochrome c for different exposure laser irradiance and excitation wavelength. We anticipate that the proposed new method will be valuable in the study of metabolic processes in mitochondria in response to low level laser exposure, and thus aid in elucidating the mechanism(s) of photobiomodulation.

  16. Resonant absorption effects induced by polarized laser ligth irradiating thin foils in the tnsa regime of ion acceleration

    International Nuclear Information System (INIS)

    Torrisi, L.; Badziak, J.; Rosinski, M.; Zaras-Szydlowska, A.; Pfeifer, M.; Torrisi, A.

    2016-01-01

    Thin foils were irradiated by short pulsed lasers at intensities of 10 16−19 W/cm 2 in order to produce non-equilibrium plasmas and ion acceleration from the target-normal-sheath-acceleration (TNSA) regime. Ion acceleration in forward direction was measured by SiC detectors and ion collectors used in the time-of-flight configuration. Laser irradiations were employed using p-polarized light at different incidence angles with respect to the target surface and at different focal distances from the target surface. Measurements demonstrate that resonant absorption effects, due to the plasma wave excitations, enhance the plasma temperature and the ion acceleration with respect to those performed without to use of p-polarized light. Dependences of the ion flux characteristics on the laser energy, wavelength, focal distance and incidence angle will be reported and discussed

  17. Effect of pulse slippage on resonant second harmonic generation of a short pulse laser in a plasma

    International Nuclear Information System (INIS)

    Nitikant; Sharma, A K

    2004-01-01

    The process of second harmonic generation of an intense short pulse laser in a plasma is resonantly enhanced by the application of a magnetic wiggler. The wiggler of suitable wave number k-vector 0 provides necessary momentum to second harmonic photons to make harmonic generation a resonant process. The laser imparts an oscillatory velocity to electrons and exerts a longitudinal ponderomotive force on them at (2ω 1 ,2k-vector 1 ), where ω 1 and k-vector 1 are the frequency and the wave number of the laser, respectively. As the electrons acquire oscillatory velocity at the second harmonic, the wiggler magnetic field beats with it to produce a transverse second harmonic current at (2ω 1 ,2k-vector 1 +k-vector 0 ), driving the second harmonic electromagnetic radiation. However, the group velocity of the second harmonic wave is greater than that of the fundamental wave, hence, the generated pulse slips out of the main laser pulse and its amplitude saturates

  18. Development of a highly sensitive lithium fluoride thermoluminescence dosimeter

    International Nuclear Information System (INIS)

    Moraes da Silva, Teresinha de; Campos, Leticia Lucente

    1995-01-01

    In recent times, LiF: Mg, Cu, P thermoluminescent phosphor has been increasingly in use for radiation monitoring due its high sensitivity and ease of preparation. The Dosimetric Materials Production Laboratory of IPEN, (Nuclear Energy Institute) has developed a simple method to obtain high sensitivity LiF. The preparation method is described. (author). 4 refs., 1 fig., 1 tab

  19. Nonlinear Label-Free Biosensing With High Sensitivity Using As2S3 Chalcogenide Tapered Fiber

    DEFF Research Database (Denmark)

    Markos, Christos; Bang, Ole

    2015-01-01

    We demonstrate an experimentally feasible fiber design, which can act as a highly sensitive, label-free, and selective biosensor using the inherent high nonlinearity of an As2S3 chalcogenide tapered fiber. The surface immobilization of the fiber with an antigen layer can provide the possibility t......, this high sensitivity can be obtained using a low-power 1064-nm microchip laser....

  20. Singly-resonant sum frequency generation of visible light in a semiconductor disk laser

    DEFF Research Database (Denmark)

    Andersen, Martin Thalbitzer; Schlosser, P.J.; Hastie, J.E.

    2009-01-01

    In this paper a generic approach for visible light generation is presented. It is based on sum frequency generation between a semiconductor disk laser and a solid-state laser, where the frequency mixing is achieved within the cavity of the semiconductor disk laser using a singlepass of the solid......-state laser light. This exploits the good beam quality and high intra-cavity power present in the semiconductor disk laser to achieve high conversion efficiency. Combining sum frequency mixing and semiconductor disk lasers in this manner allows in principle for generation of any wavelength within the visible...

  1. Numerical study of combustion initiation in a supersonic flow of H2-air mixture by resonance laser radiation

    International Nuclear Information System (INIS)

    Bezgin, L V; Kopchenov, V I; Kuleshov, P S; Titova, N S; Starik, A M

    2012-01-01

    A comparative analysis of the efficiency of approaches based on the exposure of reacting gas to resonance laser radiation to enhance combustion in a supersonic flow of H 2 -air mixture is conducted. The kinetic processes responsible for the intensification of chain reactions in premixed and non-premixed H 2 -air flows upon photodissociation of O 2 molecules by 193.3 nm laser radiation, excitation of these molecules to the singlet sigma state by laser photons with 762.346 nm wavelength and heating the mixture by laser radiation are analysed in a detailed manner. It is shown that both photochemical methods, photodissociation and excitation of O 2 molecules, are much more effective in shortening the ignition delay length than merely heating the mixture. For the premixed flow, the photodissociation of O 2 molecules ensures a slightly higher reduction in the ignition delay than the laser-induced excitation of molecular oxygen to the singlet sigma state. However, in the non-premixed flow the situation is inverted. The analysis shows that both photochemical methods make it possible to raise the efficiency of conversion of reactant chemical energy to thermal energy released during combustion compared with the method of heating the mixtures. (paper)

  2. Validation studies on quick analysis of MOX fuel by combination of laser induced breakdown spectroscopy and ablation resonance absorption spectroscopy

    International Nuclear Information System (INIS)

    Wakaida, Ikuo; Akaoka, Katsuaki; Miyabe, Masabumi; Kato, Masaaki; Otobe, Haruyoshi; Ohoba, Hironori; Khumaeni, Ali

    2014-01-01

    Research and development of laser based quick analysis without chemical analysis and neutron measurement for next-generation Minor Actinide containing MOX fuel has been carried out, and the basic performances by using un-irradiated MOX fuel were demonstrated. The glove box had been re-constructed and specialized for laser spectroscopy, and the remote spectroscopy of MOX sample contained several concentrations of Pu was performed. In elemental analysis by Laser Induced Breakdown Spectroscopy (LIBS) with high resolution spectrometer, relative error of 2.9% at 30% Pu and the detection lower limit of 2500ppm in natural U oxide were demonstrated with the operation time of 5 min. In isotope ratio analysis by Ablation Resonance Absorption Spectroscopy, tunable semiconductor laser system was constructed, and the performances such as relative deviation less than 1% in the ratio of "2"4"0Pu/"2"3"9Pu and the sensitivity of 30-100ppm in natural U were also accomplished with laser operation time of 3 to 5min. As for an elemental analysis of the simulated liquid sample, ultra-thin laminate flow was experimented as LIBS target, and the sensitivity comparable to conventional ICP-AES was confirmed. Present study includes the result of the entrusted project by the Ministry of Education, Culture, Sports, Science and Technology of Japan (MEXT). (author)

  3. The influence of wavelength, temporal sequencing, and pulse duration on resonant infrared matrix-assisted laser processing of polymer films

    Science.gov (United States)

    O'Malley, S. M.; Schoeffling, Jonathan; Jimenez, Richard; Zinderman, Brian; Yi, SunYong; Bubb, D. M.

    2014-06-01

    We have carried out a systematic investigation of laser ablation plume interactions in resonant infrared matrix-assisted pulsed laser evaporation. The laser source utilized in this study was a mid-infrared OPO capable of dual sequential ns pulses with adjustable delay ranging from 1 to 100 μs. This unique capability enabled us both to probe the ablation plume with a second laser pulse, and to effectively double the laser fluence. The primary ablation target used for this study consisted of poly(methyl methacrylate) dissolved in a binary mixture of methanol and toluene. Both the critical thermodynamic and optical properties of the binary mixture were determined and used to interpret our results. We found that deposition rates associated with single pulse irradiation tracks with the optical absorption coefficient in the spectral range from 2,700 to 3,800 nm. In the case of dual sequential pulses, discrepancies in this trend have been linked to the rate of change in the optical absorption coefficient with temperature. The influence of fluence on deposition rate was found to follow a sigmoidal dependence. Surface roughness was observed to have a diametrically opposed trend with pulse delay depending on whether the OH or CH vibrational mode was excited. In the case of CH excitation, we suggest that the rougher films are due to the absorbance of the second pulse by droplets within the plume containing residual solvent which leads to the formation of molecular balloons and hence irregularly shaped features on the substrate.

  4. Quantifying Uranium Isotope Ratios Using Resonance Ionization Mass Spectrometry: The Influence of Laser Parameters on Relative Ionization Probability

    Energy Technology Data Exchange (ETDEWEB)

    Isselhardt, Brett H. [Univ. of California, Berkeley, CA (United States)

    2011-09-01

    Resonance Ionization Mass Spectrometry (RIMS) has been developed as a method to measure relative uranium isotope abundances. In this approach, RIMS is used as an element-selective ionization process to provide a distinction between uranium atoms and potential isobars without the aid of chemical purification and separation. We explore the laser parameters critical to the ionization process and their effects on the measured isotope ratio. Specifically, the use of broad bandwidth lasers with automated feedback control of wavelength was applied to the measurement of 235U/238U ratios to decrease laser-induced isotopic fractionation. By broadening the bandwidth of the first laser in a 3-color, 3-photon ionization process from a bandwidth of 1.8 GHz to about 10 GHz, the variation in sequential relative isotope abundance measurements decreased from >10% to less than 0.5%. This procedure was demonstrated for the direct interrogation of uranium oxide targets with essentially no sample preparation. A rate equation model for predicting the relative ionization probability has been developed to study the effect of variation in laser parameters on the measured isotope ratio. This work demonstrates that RIMS can be used for the robust measurement of uranium isotope ratios.

  5. Tuneable Gaussian to flat-top resonator by amplitude beam shaping using a digital laser

    CSIR Research Space (South Africa)

    Ngcobo, S

    2014-02-01

    Full Text Available In this paper we experimentally demonstrate a simple laser cavity that produces spatial tuneable laser modes from a Gaussian beam to a Flat-top beam and a Donut-beam. The laser cavity contains an opaque ring and an adjustable circular aperture...

  6. Influence of resonator length on catastrophic optical damage in high-power AlGaInP broad-area lasers

    Science.gov (United States)

    Bou Sanayeh, Marwan

    2017-05-01

    The increasing importance of extracting high optical power out of semiconductor lasers motivated several studies in catastrophic optical damage (COD) level improvement. In this study, the influence of the resonator length in high-power broad-area (BA) AlGaInP lasers on COD is presented. For the analyses, several 638 nm AlGaInP 60 μm BA lasers from the same wafer were used. Resonator lengths of 900, 1200, 1500, and 1800 μm were compared. In order to independently examine the effect of the resonator length on the maximum power reached by the lasers before COD (PCOD), the lasers used are uncoated and unmounted, and PCOD under pulsed mode was determined. It was found that higher output powers and eventually higher PCOD can be achieved using longer resonators; however, it was also found that this is mainly useful when working at high output powers far away from the laser threshold, since the threshold current and slope efficiency worsen when the resonator length increases.

  7. V-shaped resonators for addition of broad-area laser diode arrays

    Science.gov (United States)

    Liu, Bo; Liu, Yun; Braiman, Yehuda Y.

    2012-12-25

    A system and method for addition of broad-area semiconductor laser diode arrays are described. The system can include an array of laser diodes, a V-shaped external cavity, and grating systems to provide feedback for phase-locking of the laser diode array. A V-shaped mirror used to couple the laser diode emissions along two optical paths can be a V-shaped prism mirror, a V-shaped stepped mirror or include multiple V-shaped micro-mirrors. The V-shaped external cavity can be a ring cavity. The system can include an external injection laser to further improve coherence and phase-locking.

  8. Energy spectrum and thermal properties of a terahertz quantum-cascade laser based on the resonant-phonon depopulation scheme

    Energy Technology Data Exchange (ETDEWEB)

    Khabibullin, R. A., E-mail: khabibullin@isvch.ru; Shchavruk, N. V.; Klochkov, A. N.; Glinskiy, I. A.; Zenchenko, N. V.; Ponomarev, D. S.; Maltsev, P. P. [Russian Academy of Sciences, Institute of Ultrahigh Frequency Semiconductor Electronics (Russian Federation); Zaycev, A. A. [National Research University of Electronic Technology (MIET) (Russian Federation); Zubov, F. I.; Zhukov, A. E.; Cirlin, G. E.; Alferov, Zh. I. [Russian Academy of Sciences, Saint Petersburg Academic University—Nanotechnology Research and Education Center (Russian Federation)

    2017-04-15

    The dependences of the electronic-level positions and transition oscillator strengths on an applied electric field are studied for a terahertz quantum-cascade laser (THz QCL) with the resonant-phonon depopulation scheme, based on a cascade consisting of three quantum wells. The electric-field strengths for two characteristic states of the THz QCL under study are calculated: (i) “parasitic” current flow in the structure when the lasing threshold has not yet been reached; (ii) the lasing threshold is reached. Heat-transfer processes in the THz QCL under study are simulated to determine the optimum supply and cooling conditions. The conditions of thermocompression bonding of the laser ridge stripe with an n{sup +}-GaAs conductive substrate based on Au–Au are selected to produce a mechanically stronger contact with a higher thermal conductivity.

  9. CrossRef Large numbers of cold positronium atoms created in laser-selected Rydberg states using resonant charge exchange

    CERN Document Server

    McConnell, R; Kolthammer, WS; Richerme, P; Müllers, A; Walz, J; Grzonka, D; Zielinski, M; Fitzakerley, D; George, MC; Hessels, EA; Storry, CH; Weel, M

    2016-01-01

    Lasers are used to control the production of highly excited positronium atoms (Ps*). The laser light excites Cs atoms to Rydberg states that have a large cross section for resonant charge-exchange collisions with cold trapped positrons. For each trial with 30 million trapped positrons, more than 700 000 of the created Ps* have trajectories near the axis of the apparatus, and are detected using Stark ionization. This number of Ps* is 500 times higher than realized in an earlier proof-of-principle demonstration (2004 Phys. Lett. B 597 257). A second charge exchange of these near-axis Ps* with trapped antiprotons could be used to produce cold antihydrogen, and this antihydrogen production is expected to be increased by a similar factor.

  10. Isomer separation of $^{70g}Cu$ and $^{70m}Cu$ with a resonance ionization laser ion source

    CERN Document Server

    Köster, U; Mishin, V I; Weissman, L; Huyse, M; Kruglov, K; Müller, W F; Van Duppen, P; Van Roosbroeck, J; Thirolf, P G; Thomas, H C; Weisshaar, D W; Schulze, W; Borcea, R; La Commara, M; Schatz, H; Schmidt, K; Röttger, S; Huber, G; Sebastian, V; Kratz, K L; Catherall, R; Georg, U; Lettry, Jacques; Oinonen, M; Ravn, H L; Simon, H

    2000-01-01

    Radioactive copper isotopes were ionized with the resonance ionization laser ion source at the on-line isotope separator ISOLDE (CERN). Using the different hyperfine structure in the 3d/sup 10/ 4s /sup 2/S/sub 1/2/-3d/sup 10/ 4p /sup 2/P/sub 1/2//sup 0/ transition the low- and high-spin isomers of /sup 70/Cu were selectively enhanced by tuning the laser wavelength. The light was provided by a narrow-bandwidth dye laser pumped by copper vapor lasers and frequency doubled in a BBO crystal. The ground state to isomeric state intensity ratio could be varied by a factor of 30, allowing to assign gamma transitions unambiguously to the decay of the individual isomers. It is shown that the method can also be used to determine magnetic moments. In a first experiment for the 1/sup +/ ground state of /sup 70/Cu a magnetic moment of (+)1.8(3) mu /sub N/ and for the high-spin isomer of /sup 70/Cu a magnetic moment of (+or-)1.2(3) mu /sub N/ could be deduced. (20 refs).

  11. Design and Analysis of Enhanced Modulation Response in Integrated Coupled Cavities DBR Lasers Using Photon-Photon Resonance

    Directory of Open Access Journals (Sweden)

    Paolo Bardella

    2016-01-01

    Full Text Available In the last few decades, various solutions have been proposed to increase the modulation bandwidth and, consequently, the transmission bit-rate of semiconductor lasers. In this manuscript, we discuss a design procedure for a recently proposed laser cavity realized with the monolithic integration of two distributed Bragg reflector (DBR lasers allowing one to extend the modulation bandwidth. Such an extension is obtained introducing in the dynamic response a photon-photon resonance (PPR at a frequency higher than the modulation bandwidth of the corresponding single-section laser. Design guidelines will be proposed, and dynamic small and large signal simulations results, calculated using a finite difference traveling wave (FDTW numerical simulator, will be discussed to confirm the design results. The effectiveness of the design procedure is verified in a structure with PPR frequency at 35 GHz allowing one to obtain an open eye diagram for a non-return-to-zero (NRZ digital signal up to 80 GHz . Furthermore, the investigation of the rich dynamics of this structure shows that with proper bias conditions, it is possible to obtain also a tunable self-pulsating signal in a frequency range related to the PPR design.

  12. Silicon on-chip bandpass filters for the multiplexing of high sensitivity photonic crystal microcavity biosensors

    International Nuclear Information System (INIS)

    Yan, Hai; Zou, Yi; Yang, Chun-Ju; Chakravarty, Swapnajit; Wang, Zheng; Tang, Naimei; Chen, Ray T.; Fan, Donglei

    2015-01-01

    A method for the dense integration of high sensitivity photonic crystal (PC) waveguide based biosensors is proposed and experimentally demonstrated on a silicon platform. By connecting an additional PC waveguide filter to a PC microcavity sensor in series, a transmission passband is created, containing the resonances of the PC microcavity for sensing purpose. With proper engineering of the passband, multiple high sensitivity PC microcavity sensors can be integrated into microarrays and be interrogated simultaneously between a single input and a single output port. The concept was demonstrated with a 2-channel L55 PC biosensor array containing PC waveguide filters. The experiment showed that the sensors on both channels can be monitored simultaneously from a single output spectrum. Less than 3 dB extra loss for the additional PC waveguide filter is observed

  13. Silicon on-chip bandpass filters for the multiplexing of high sensitivity photonic crystal microcavity biosensors

    Energy Technology Data Exchange (ETDEWEB)

    Yan, Hai, E-mail: hai.yan@utexas.edu; Zou, Yi; Yang, Chun-Ju [Department of Electrical and Computer Engineering, Microelectronics Research Center, The University of Texas at Austin, 10100 Burnet Rd., Austin, Texas 78758 (United States); Chakravarty, Swapnajit, E-mail: swapnajit.chakravarty@omegaoptics.com [Omega Optics, Inc., 8500 Shoal Creek Blvd., Austin, Texas 78757 (United States); Wang, Zheng [Department of Electrical and Computer Engineering, Microelectronics Research Center, The University of Texas at Austin, 10100 Burnet Rd., Austin, Texas 78758 (United States); Materials Science and Engineering Program, Texas Materials Institute, The University of Texas at Austin, Austin, Texas 78712 (United States); Tang, Naimei; Chen, Ray T., E-mail: raychen@uts.cc.utexas.edu [Department of Electrical and Computer Engineering, Microelectronics Research Center, The University of Texas at Austin, 10100 Burnet Rd., Austin, Texas 78758 (United States); Omega Optics, Inc., 8500 Shoal Creek Blvd., Austin, Texas 78757 (United States); Fan, Donglei [Materials Science and Engineering Program, Texas Materials Institute, The University of Texas at Austin, Austin, Texas 78712 (United States); Department of Mechanical Engineering, The University of Texas at Austin, Austin, Texas 78712 (United States)

    2015-03-23

    A method for the dense integration of high sensitivity photonic crystal (PC) waveguide based biosensors is proposed and experimentally demonstrated on a silicon platform. By connecting an additional PC waveguide filter to a PC microcavity sensor in series, a transmission passband is created, containing the resonances of the PC microcavity for sensing purpose. With proper engineering of the passband, multiple high sensitivity PC microcavity sensors can be integrated into microarrays and be interrogated simultaneously between a single input and a single output port. The concept was demonstrated with a 2-channel L55 PC biosensor array containing PC waveguide filters. The experiment showed that the sensors on both channels can be monitored simultaneously from a single output spectrum. Less than 3 dB extra loss for the additional PC waveguide filter is observed.

  14. A high-sensitivity neutron counter and waste-drum counting with the high-sensitivity neutron instrument

    International Nuclear Information System (INIS)

    Hankins, D.E.; Thorngate, J.H.

    1993-04-01

    At Lawrence Livermore National Laboratory (LLNL), a highly sensitive neutron counter was developed that can detect and accurately measure the neutrons from small quantities of plutonium or from other low-level neutron sources. This neutron counter was originally designed to survey waste containers leaving the Plutonium Facility. However, it has proven to be useful in other research applications requiring a high-sensitivity neutron instrument

  15. Effects of resonator input power on Kerr lens mode-locked lasers

    Indian Academy of Sciences (India)

    lasers. S KAZEMPOUR, A KESHAVARZ∗ and G HONARASA. Department of Physics, Faculty of Sciences, Shiraz University of Technology, Shiraz, Iran ... Keywords. Femtosecond pulses; Kerr lens sensitivity; Kerr lens mode-locked laser. ... The optical lengths of Kerr medium with thickness d and refractive index n under.

  16. Laser irradiations of advanced targets promoting absorption resonance for ion acceleration in TNSA regime

    Czech Academy of Sciences Publication Activity Database

    Torrisi, L.; Calcagno, L.; Giulietti, D.; Cutroneo, Mariapompea; Zimbone, M.; Skála, Jiří

    2015-01-01

    Roč. 355, JUL (2015), s. 221-226 ISSN 0168-583X Institutional support: RVO:68378271 ; RVO:61389005 Keywords : "p"-polarization * laser-generated plasma * TNSA regtime * ion acceleration in plasma Subject RIV: BG - Nuclear, Atomic and Molecular Physics, Colliders; BH - Optics, Masers, Lasers (FZU-D) Impact factor: 1.389, year: 2015

  17. Characterization of a Continuous Wave Laser for Resonance Ionization Mass Spectroscopy Analysis in Nuclear Forensics

    Science.gov (United States)

    2015-06-01

    multimode_optical_fiber. [15] J. Hecht, The Laser Guidebook, 2nd ed, Blue Ride Summit, PA: Mc Graw Hill Professional, 1999, pp. 101–109. [16] F...Available: https://secure.sacher-laser.com/downloads/- technical_documents/t03d6w-en.pdf. [22] J. H. Marquardt, F. C. Cruz, M. Stephens , C. W. Oates

  18. Development of an optical resonator with high-efficient output coupler for the JAERI far-infrared free-electron laser

    International Nuclear Information System (INIS)

    Nagai, Ryoji; Hajima, Ryoichi; Nishimori, Nobuyuki; Sawamura, Masaru; Kikuzawa, Nobuhiro; Shizuma, Toshiyuki; Minehara, Eisuke

    2001-01-01

    An optical resonator with a high-efficient output coupler was developed for the JAERI far-infrared free-electron laser. The optical resonator is symmetrical near-concentric geometry with an insertable scraper output coupler. As a result of the development of the optical resonator, the JAERI-FEL has been successfully, lased with averaged power over 1 kW. Performance of the optical resonator with the output coupler was evaluated at optical wavelength of 22 μm by using an optical mode calculation code. The output coupling and diffractive loss with a dominant eigen-mode of the resonator were calculated using an iterative computation called Fox-Li procedure. An efficiency factor of the optical resonator was introduced for the evaluation of the optical resonator performance. The efficiency factor was derived by the amount of the output coupling and diffractive loss of the optical resonator. It was found that the optical resonator with the insertable scraper coupler was the most suitable to a high-power and high-efficient far-infrared free-electron laser. (author)

  19. High sensitivity detection of desorbed biomolecules by photoionization with tunable VUV

    International Nuclear Information System (INIS)

    Moore, J.F.; Calaway, W.F.; Veryovkin, I.V.; Pellin, M.J.; Lewellen, J.W.; Li, Y.; Milton, S.V.; King, B.V.

    2004-01-01

    Full text: The spectral region from 7 to 11eV has two attributes that make it attractive for biomolecule photoionization: 1. high photoionization cross sections, leading to high detection efficiency, and 2. overlap with nearly all first ionization energies of biomolecules, allowing possible control over fragmentation by accessing different final states via tuning. The lack of available tunable lasers in this energy range has generally hindered exploitation of these features thus far. A free-electron laser in operation at Argonne National Laboratory provides high pulse energy, widely tunable VUV pulses of 300 fs duration. Coupled with a novel time-of-flight mass spectrometer, this laser is able to photoionize and detect biomolecules, including peptides and nucleosides. Either laser desorption or primary ion beams are used to desorb sample material, followed by photoionization with a VUV laser. The instrument uses novel ion optics to extract photoions from a large volume while maintaining high mass resolution. This approach is capable of yielding dramatically improved detection limits over more conventional methods such as MALDI and SIMS. In the case of the common peptide substance P, for example, a substantial improvement over the MALDI signal was observed using VUV photoionization with very little observed fragmentation of the molecule. Nucleosides and cisplatin were also measured with typically order of magnitude improvements in signal. These and other examples show clearly the benefits that can be obtained in high sensitivity mass spectrometry of biomolecules with the increasing availability of VUV laser sources

  20. VUV optical ring resonator for Duke storage ring free electron laser

    Energy Technology Data Exchange (ETDEWEB)

    Park, S.H.; Litvinenko, V.N.; Madey, J.M.J. [Duke Univ., Durham, NC (United States)] [and others

    1995-12-31

    The conceptual design of the multifaceted-mirror ring resonator for Duke storage ring VUV FEL is presented. The expected performance of the OK-4 FEL with ring resonator is described. We discuss in this paper our plans to study reflectivity of VUV mirrors and their resistivity to soft X-ray spontaneous radiation from OK-4 undulator.

  1. Multiphoton resonances

    International Nuclear Information System (INIS)

    Shore, B.W.

    1977-01-01

    The long-time average of level populations in a coherently-excited anharmonic sequence of energy levels (e.g., an anharmonic oscillator) exhibits sharp resonances as a function of laser frequency. For simple linearly-increasing anharmonicity, each resonance is a superposition of various multiphoton resonances (e.g., a superposition of 3, 5, 7, . . . photon resonances), each having its own characteristic width predictable from perturbation theory

  2. Production of high-power CW UV by resonant frequency quadrupling of a Nd:YLF laser

    International Nuclear Information System (INIS)

    Kuczewski, A.J.; Thorn, C.E.

    1999-01-01

    The authors have constructed a single ring to resonantly double an 18 watt Nd:YLF mode-locked laser and re-double the stored green to produce over 4 watts of power in the ultra-violet (UV). This laser is used to produce a beam of 470 MeV gamma-rays by Compton backscattering the laser beam from 2.8 GeV electrons stored in a synchrotron. Achieving high luminosity of the colliding beams requires very good mode quality and beam stability at the intersection point 22 meters from the laser. The ring consists of six mirrors, with two 25 cm radius of curvature mirrors enclosing each nonlinear crystal. The drive laser is a lamp-pumped Nd:YLF with a 50 ps bunch length at 76 MHz. A pointing stabilizer servo has been constructed as part of the infrared (IR) mode matching telescope. The IR to green conversion is accomplished in a 15 mm long non-critically phased matched LBO crystal located at a 40 micron waist, with an IR conversion efficiency of 70%. A stable, nearly diffraction limited UV beam of up to 4.2 watts is generated in a BBO crystal in the green storage ring. The output power is relatively independent of the efficiency of the LBO and BBO crystals. This fact makes it possible to reduce the amount of non-TEM 00 modes created by walk-off of the UV by using relatively thin BBO crystals. At present, however, the lower bound on the BBO thickness is limited by the loss of conversion efficiency at high power

  3. Parametric resonance in superconducting micron-scale waveguides

    International Nuclear Information System (INIS)

    Fomin, N.V.; Shalaev, O.L.; Shantsev, D.V.

    1997-01-01

    A parametric resonance due to temperature oscillations in superconducting micron-scale waveguides is considered. Oscillations of superconductor temperature are assumed to be induced by the irradiation of the waveguide with a laser beam. The laser power and parameters of the waveguide providing a possibility of parametric excitation have been calculated. It is shown that for a waveguide made of a YBa 2 Cu 3 O 7 microstrip with resonant frequency of 10 GHz a laser with a power of about 70 W/cm 2 is needed to excite oscillations. The effect can be used for the creation of high-sensitivity tuneable filters and optoelectric transformers on superconducting microstrips in the GHz range. copyright 1997 American Institute of Physics

  4. Quantum averaging and resonances: two-level atom in a one-mode classical laser field

    Directory of Open Access Journals (Sweden)

    M. Amniat-Talab

    2007-06-01

    Full Text Available   We use a nonperturbative method based on quantum averaging and an adapted from of resonant transformations to treat the resonances of the Hamiltonian of a two-level atom interacting with a one-mode classical field in Floquet formalism. We illustrate this method by extraction of effective Hamiltonians of the system in two regimes of weak and strong coupling. The results obtained in the strong-coupling regime, are valid in the whole range of the coupling constant for the one-photon zero-field resonance.

  5. Electron scattering by an atom in the field of resonant laser radiation

    International Nuclear Information System (INIS)

    Agre, M.; Rapoport, L.

    1982-01-01

    The collision of an electron with an atom in the field of intense electromagnetic radiation that is at resonance with two atomic multiplets is investigated theoretically. Expressions are obtained for the amplitudes of the elastic and inelastic scattering with emission (absorption) of photons. The case of a ground state at resonance with a doublet is considered in detail. It is shown that photon absorption takes place predominantly in the case of resonance in inelastic transitions from a state of the lower multiplet, and photon emission takes place in transitions from a state of the upper multiplet

  6. Highly sensitive heavy metal ion detection using AlQ3 microwire functionalized QCM

    Science.gov (United States)

    Can, Nursel; Aǧar, Meltem; Altındal, Ahmet

    2016-03-01

    Tris(8-hydroxyquinoline) aluminum (Alq3) microwires was successfully synthesized for the fabrication of Alq3 microwires-coated QCM sensors to detect the heavy metal ions in aqueous solution. AT-cut quartz crystal microbalance (QCM) of 10 MHz fundamental resonance frequency having gold electrodes were used as transducers. Typical measuring cycle consisted of repeated flow of target measurands through the flow cell and subsequent washing to return the baseline. The QCM results indicated that the Alq3 microwires exhibit excellent sensitivity, stability and short response-recovery time, which are much attractive for the development of portable and highly sensitive heavy metal ion sensors in water samples.

  7. Creating geometrically robust designs for highly sensitive problems using topology optimization: Acoustic cavity design

    DEFF Research Database (Denmark)

    Christiansen, Rasmus E.; Lazarov, Boyan S.; Jensen, Jakob S.

    2015-01-01

    Resonance and wave-propagation problems are known to be highly sensitive towards parameter variations. This paper discusses topology optimization formulations for creating designs that perform robustly under spatial variations for acoustic cavity problems. For several structural problems, robust...... and limitations are discussed. In addition, a known explicit penalization approach is considered for comparison. For near-uniform spatial variations it is shown that highly robust designs can be obtained using the double filter approach. It is finally demonstrated that taking non-uniform variations into account...... further improves the robustness of the designs....

  8. Resonant Laser Ignition Study of HAN-HEHN Propellant Mixture (Preprint)

    National Research Council Canada - National Science Library

    Alfano, Angelo J; Mills, Jeffrey D; Vaghjiani, Ghanshyam L

    2008-01-01

    ...) - hydroxyethylhydrazinium nitrate (HEHN) mixtures. This prototypical ionic liquid propellant was successfully and reliably ignited/detonated under confinement with single laser pulses in the mid IR at 2.94 and 10.6 microns...

  9. Probing ultrafast changes of spin and charge density profiles with resonant XUV magnetic reflectivity at the free-electron laser FERMI.

    Science.gov (United States)

    Gutt, C; Sant, T; Ksenzov, D; Capotondi, F; Pedersoli, E; Raimondi, L; Nikolov, I P; Kiskinova, M; Jaiswal, S; Jakob, G; Kläui, M; Zabel, H; Pietsch, U

    2017-09-01

    We report the results of resonant magnetic XUV reflectivity experiments performed at the XUV free-electron laser FERMI. Circularly polarized XUV light with the photon energy tuned to the Fe M 2,3 edge is used to measure resonant magnetic reflectivities and the corresponding Q -resolved asymmetry of a Permalloy/Ta/Permalloy trilayer film. The asymmetry exhibits ultrafast changes on 240 fs time scales upon pumping with ultrashort IR laser pulses. Depending on the value of the wavevector transfer Q z , we observe both decreasing and increasing values of the asymmetry parameter, which is attributed to ultrafast changes in the vertical spin and charge density profiles of the trilayer film.

  10. Amplification of an Autodyne Signal in a Bistable Vertical-Cavity Surface-Emitting Laser with the Use of a Vibrational Resonance

    Science.gov (United States)

    Chizhevsky, V. N.

    2018-01-01

    For the first time, it is demonstrated experimentally that a vibrational resonance in a polarization-bistable vertical-cavity surface-emitting laser can be used to increase the laser response in autodyne detection of microvibrations from reflecting surfaces. In this case, more than 25-fold signal amplification is achieved. The influence of the asymmetry of the bistable potential on the microvibration-detection efficiency is studied.

  11. Enhanced off-resonance magnetoelectric response in laser annealed PZT thick film grown on magnetostrictive amorphous metal substrate

    Energy Technology Data Exchange (ETDEWEB)

    Palneedi, Haribabu [Materials Interface Laboratory, Department of Materials Science and Engineering, Korea Advanced Institute of Science and Technology (KAIST), Daejeon 305-701 (Korea, Republic of); Functional Ceramics Group, Korea Institute of Materials Science (KIMS), Changwon 641-831 (Korea, Republic of); Maurya, Deepam; Priya, Shashank [Bio-inspired Materials and Devices Laboratory (BMDL), Center for Energy Harvesting Materials and Systems (CEHMS), Virginia Tech, Blacksburg, Virginia 24061 (United States); Kim, Gi-Yeop; Choi, Si-Young, E-mail: youngchoi@kims.re.kr [Materials Modeling and Characterization Department, Korea Institute of Materials Science (KIMS), Changwon 641-831 (Korea, Republic of); Kang, Suk-Joong L. [Materials Interface Laboratory, Department of Materials Science and Engineering, Korea Advanced Institute of Science and Technology (KAIST), Daejeon 305-701 (Korea, Republic of); Kim, Kwang-Ho [School of Materials Science and Engineering, Pusan National University, Busan 609-735 (Korea, Republic of); Ryu, Jungho, E-mail: jhryu@kims.re.kr [Functional Ceramics Group, Korea Institute of Materials Science (KIMS), Changwon 641-831 (Korea, Republic of)

    2015-07-06

    A highly dense, 4 μm-thick Pb(Zr,Ti)O{sub 3} (PZT) film is deposited on amorphous magnetostrictive Metglas foil (FeBSi) by granule spray in vacuum process at room temperature, followed by its localized annealing with a continuous-wave 560 nm ytterbium fiber laser radiation. This longer-wavelength laser radiation is able to anneal the whole of thick PZT film layer without any deteriorative effects, such as chemical reaction and/or atomic diffusion, at the interface and crystallization of amorphous Metglas substrate. Greatly enhanced dielectric and ferroelectric properties of the annealed PZT are attributed to its better crystallinity and grain growth induced by laser irradiation. As a result, a colossal off-resonance magnetoelectric (ME) voltage coefficient that is two orders of magnitude larger than previously reported output from PZT/Metglas film-composites is achieved. The present work addresses the problems involved in the fabrication of PZT/Metglas film-composites and opens up emerging possibilities in employing piezoelectric materials with low thermal budget substrates (suitable for integrated electronics) and designing laminate composites for ME based devices.

  12. Extremely-high vacuum pressure measurement by laser ionization

    International Nuclear Information System (INIS)

    Kokubun, Kiyohide

    1991-01-01

    Laser ionization method has the very high sensitivity for detecting atoms and molecules. Hurst et al. successfully detected a single Cs atom by means of resonance ionization spectroscopy developed by them. Noting this high sensitivity, the authors have attempted to apply the laser ionization method to measure gas pressure, particularly in the range down to extremely high vacuum. At present, hot cathode ionization gauges are used for measuring gas pressure down to ultrahigh vacuum, however, those have a number of disadvantages. The pressure measurement using lasers does not have such disadvantages. The pressure measurement utilizing the laser ionization method is based on the principle that when laser beam is focused through a lens, the amount of atom or molecule ions generated in the focused space region is proportional to gas pressure. In this paper, the experimental results are presented on the nonresonant multiphoton ionization characteristics of various kinds of gases, the ion detection system with high sensitivity and an extremely high vacuum system prepared for the laser ionization experiment. (K.I.)

  13. Rapid vibrational and rotational energy-transfer rates in heated carbon dioxide collisions by double-resonance laser spectroscopy

    International Nuclear Information System (INIS)

    Thomason, M.D.

    1982-07-01

    Rates for resonant vibrational and rotational energy transfer from the 001 state by CO 2 + CO 2 collisions have been measured. All data were obtained by double resonance spectroscopy with CO 2 lasers in a 2.5 meter absorption cell at 700 0 K. Results for rotation transfer include pumped-level relaxation and the response of other 001 levels with ΔJ up to 18. These data are compared to four relevant collision models via a 35-level rate equation analysis. Sequence-band (002 → 101) and hot-band (011 → 110) lasting have been used to observe resonant nu 3 -transfer relaxation involving 001 + 001 reversible 002 + 000, 001 + 100 reversible 101 + 000, and 001 + 010 reversible 011 + 000. A multilevel rate analysis has been utilized to determine the rate coefficients for 001 going to the 002, the 101, and the 011 levels. Part of the hot-band data has been interpreted as due to 110 + 000 reversible 100 + 010, and the associated rate constant has been estimated. The results of the study are compared to the theory and to other experiments

  14. Reactions of metal ions and their clusters in the gas phase using laser ionization: ion cyclotron resonance spectroscopy

    International Nuclear Information System (INIS)

    Freiser, B.S.

    1981-04-01

    Two subjects are discussed in this report: advances in proposed studies on metal ion chemistry and expansion of laboratory facilities. The development of a combined pulsed laser source-ion cyclotron resonance spectrometer has proven to be a convenient and powerful method for generating metal ions and for studying their subsequent chemistry in the gas phase. The main emphasis of this research has been on the application of metal ions as a selective chemical ionization reagents and progress in this area are discussed. The goal is to identify trends in reactivity i.e. mechanisms useful in interpreting the chemical ionization spectra of unknown compounds and to test for the functional group selectivity of the various metal ions. The feasibility of these goals have been demonstrated in extensive studies on Cu + with esters and ketones, on Fe + with ethers, ketones, and hydrocarbons, and on Ti + with hydrocarbons. In addition, preliminary results on sulfur containing compounds and on a variety of other metallic ions have been obtained. Laboratory facilities were expanded from one ion cyclotron resonance (ICR) spectrometer to two, plus a third instrument the Fourier Transform Ion Cyclotron Resonance (FTICR) spectrometer

  15. Optimization of electrodynamic characteristics of the buncher-resonator for a free electron laser

    International Nuclear Information System (INIS)

    Sobenin, N.P.; Kalyuzhnyj, V.E.; Kostin, D.V.; Yarygin, S.N.; Zavadtsev, A.A.

    1994-01-01

    Selection of geometric sizes of a resonator buncher comprising 1.5 accelerating cells and linking cell is performed. When selecting the inner resonator dimensions the attention is first of all paid to minimization of E r /E z (z, γ) function in the axial region. At the same time the value of the field overstrain coefficient under a high value of effective shunt resistance is also minimized at the expense of changing the drift tube profile. 2 refs.; 2 figs.; 4 tabs

  16. Production of radioactive ion beams and resonance ionization spectroscopy with the laser ion source at on-line isotope separator ISOLDE

    International Nuclear Information System (INIS)

    Fedosseev, V.N.; )

    2005-01-01

    Full text: The resonance ionisation laser ion source (RILIS) of the ISOLDE on-line isotope separation facility at CERN is based on the method of laser step-wise resonance ionisation of atoms in a hot metal cavity. Using the system of dye lasers pumped by copper vapour lasers the ion beams of many different metallic elements have been produced at ISOLDE with an ionization efficiency of up to 27%. The high selectivity of the resonance ionization is an important asset for the study of short-lived nuclides produced in targets bombarded by the proton beam of the CERN Booster accelerator. Radioactive ion beams of Be, Mg, Al, Mn, Ni, Cu, Zn, Ga, Ag, Cd, In, Sn, Sb, Tb, Yb, Tl, Pb and Bi have been generated with the RILIS. Setting the RILIS laser in the narrow line-width mode provides conditions for a high-resolution study of hyperfine structure and isotopic shifts of atomic lines for short-lived isotopes. The isomer selective ionization of Cu, Ag and Pb isotopes has been achieved by appropriate tuning of laser wavelengths

  17. Aluminum nano-cantilevers for high sensitivity mass sensors

    DEFF Research Database (Denmark)

    Davis, Zachary James; Boisen, Anja

    2005-01-01

    We have fabricated Al nano-cantilevers using a very simple one mask contact UV lithography technique with lateral dimensions under 500 nm and vertical dimensions of approximately 100 nm. These devices are demonstrated as highly sensitive mass sensors by measuring their dynamic properties. Further...

  18. Laser surface modification of medical grade alloys for reduced heating in a magnetic resonance imaging environment

    Energy Technology Data Exchange (ETDEWEB)

    Benafan, O., E-mail: othmane.benafan@nasa.gov, E-mail: raj@ucf.edu; Vaidyanathan, R., E-mail: othmane.benafan@nasa.gov, E-mail: raj@ucf.edu [Advanced Materials Processing and Analysis Center (AMPAC), Materials Science and Engineering, Mechanical and Aerospace Engineering, University of Central Florida, Orlando, Florida 32816 (United States); Chen, S.-Y.; Kar, A. [Laser-Advanced Materials Processing Laboratory, Center for Research and Education in Optics and Lasers (CREOL), College of Optics and Photonics, University of Central Florida, Orlando, Florida 32816 (United States)

    2015-12-15

    Nanoscale surface modification of medical grade metallic alloys was conducted using a neodymium-doped yttrium aluminum garnet laser-based dopant diffusion technique. The objective of this approach was to minimize the induction heating by reducing the absorbed radio frequency field. Such an approach is advantageous in that the dopant is diffused into the alloy and is not susceptible to detachment or spallation as would an externally applied coating, and is expected to not deteriorate the mechanical and electrical properties of the base alloy or device. Experiments were conducted using a controlled environment laser system with the ability to control laser properties (i.e., laser power, spot size, and irradiation time) and dopant characteristics (i.e., temperature, concentration, and pressure). The reflective and transmissive properties of both the doped and untreated samples were measured in a radio frequency (63.86 MHz) magnetic field using a system comprising a high power signal generator, a localized magnetic field source and sensor, and a signal analyzer. The results indicate an increase in the reflectivity of the laser-treated samples compared to untreated samples. The effect of reflectivity on the heating of the alloys is investigated through a mathematical model incorporating Maxwell’s equations and heat conduction.

  19. The identification of autoionizing states of atomic chromium for the resonance ionization laser ion source of the ISOLDE radioactive ion beam facility

    CERN Document Server

    Goodacre, T Day

    2017-01-01

    The resonance ionization laser ion source (RILIS) is the principal ion source of the ISOLDE radioactive beam facility based at CERN. Using the method of in-source resonance ionization spectroscopy, an optimal three-step, three-resonance photo-ionization scheme has been developed for chromium. The scheme uses an ionizing transition to one of the 14 newly observed autoionizing states. This work increases the range of ISOLDE-RILIS ionized beams to 32 chemical elements. Details of the spectroscopic studies are described and the new ionization scheme is summarized. A link to the complete version of this document will be added here following publication:

  20. Anomalous intensities of Ne-like ion resonance line in plasma produced by picosecond laser pulse

    International Nuclear Information System (INIS)

    Bryunetkin, B.A.; Skobelev, I.Yu.; Faenov, A.Ya.; Kalashnikov, M.P.; Nikles, P.; Shnyupep, M.

    1995-01-01

    An anomalous structure of intensities of spectral lines of CuXX and GeXXX Ne-like ions emitted by plasma produced by laser pulses of picosecond duration and up to 2x10 18 W/cm 2 flux density is recorded for the first time. It is shown that spectrum maximum of these ions is emitted from a plasma region whose density is significantly above the critical value of the length of heating laser radiation wave. 9 refs.; 3 figs

  1. Stability of a Short Rayleigh Range Laser Resonator with Misaligned or Distorted Mirrors

    CERN Document Server

    Crooker, Peter P; Colson, William B

    2004-01-01

    Motivated by the prospect of constructing an FEL with short Rayleigh length in a high-vibration shipboard environment, we have studied the effect of mirror vibration and distortion on the behavior of the fundamental optical mode of a cold-cavity resonator. A tilt or transverse shift of a mirror causes the optical mode to rock sinusoidally about the original resonator axis. A longitudinal mirror shift or a change in the mirror’s radius of curvature causes the beam diameter at a mirror to dilate and contract with successive impacts. Results from both ray-tracing techniques and wavefront propagation simulations are in excellent agreement.

  2. Characterization of non-polar aromatic hydrocarbons in crude oil using atmospheric pressure laser ionization and Fourier transform ion cyclotron resonance mass spectrometry (APLI FT-ICR MS).

    Science.gov (United States)

    Schrader, Wolfgang; Panda, Saroj K; Brockmann, Klaus J; Benter, Thorsten

    2008-07-01

    We report on the successful application of the recently introduced atmospheric pressure laser ionization (APLI) method as a novel tool for the analysis of crude oil and its components. Using Fourier transform ion cyclotron resonance mass spectrometry, unambiguous determination of key compounds in this complex matrix with unprecedented sensitivity is presented.

  3. Laser photo-reflectance characterization of resonant nonlinear electro-refraction in thin semiconductor films

    International Nuclear Information System (INIS)

    Chism, Will; Cartwright, Jason

    2012-01-01

    Photo-reflectance (PR) measurements provide a non-contact means for the precise characterization of semiconductor electronic properties. In this paper, we investigate the use of a laser beam as the probe beam in the PR setup. In this case it is seen that the nonlinear refraction is responsible for the amplitude change of the reflected probe field, whereas the phase change is due to nonlinear absorption. The open aperture condition may then be used to eliminate the spatial phase at the detector, thereby isolating the electro-refractive contribution to the PR signal. This greatly simplifies the PR analysis and allows absolute measurements of electro-refraction in thin semiconductor films. We report the application of the laser PR technique to characterize physical strain in thin silicon on silicon-germanium films. - Highlights: ► We describe the theory of laser photoreflectance. ► Laser photoreflectance is used to independently characterize nonlinear refraction. ► We report the characterization of strain in thin strained silicon films.

  4. Evolution of Wigner function in laser process under the action of linear resonance force and its application

    Science.gov (United States)

    Dao-ming, Lu

    2018-05-01

    The negativity of Wigner function (WF) is one of the important symbols of non-classical properties of light field. Therefore, it is of great significance to study the evolution of WF in dissipative process. The evolution formula of WF in laser process under the action of linear resonance force is given by virtue of thermo entangled state representation and the technique of integration within an ordered product of operator. As its application, the evolution of WF of thermal field and that of single-photon-added coherent state are discussed. The results show that the WF of thermal field maintains its original character. On the other hand, the negative region size and the depth of negativity of WF of single- photon-added coherent state decrease until it vanishes with dissipation. This shows that the non-classical property of single-photon-added coherent state is weakened, until it disappears with dissipation time increasing.

  5. Trace isotope analysis using resonance ionization mass spectrometry based on isotope selection with doppler shift of laser ablated atoms

    International Nuclear Information System (INIS)

    Higuchi, Yuki; Watanabe, Kenichi; Kawarabayashi, Jun; Iguchi, Tetsuo

    2005-01-01

    We have proposed a novel isotope selective Resonance Ionization Mass Spectroscopy (RIMS) concept, which can avoid the Doppler broadening on solid sample direct measurement based on laser ablation technique. We have succeeded in experimentally demonstrating the principle of our RIMS concept. Through comparison between the simulated and experimental results, we have validated the simulation model. It would be concluded from these results that we could achieve the isotope selectivity defined as the ratio of 41 Ca to 40 Ca sensitivity to be 4.5x10 10 by adopting the multi-step excitation scheme in the present method. As future works, we will try to experimentally perform the multi-step excitation scheme and improve the detection efficiency by modifying the ion extraction configuration. (author)

  6. Resonant laser power build-up in ALPS-A 'light shining through a wall' experiment

    Energy Technology Data Exchange (ETDEWEB)

    Ehret, Klaus [Deutsches Elektronen-Synchrotron DESY, Notkestrasse 85, D-22607 Hamburg (Germany); Frede, Maik [Laser Zentrum Hannover e.V., Hollerithallee 8, D-30419 Hannover (Germany); Ghazaryan, Samvel [Deutsches Elektronen-Synchrotron DESY, Notkestrasse 85, D-22607 Hamburg (Germany); Hildebrandt, Matthias [Laser Zentrum Hannover e.V., Hollerithallee 8, D-30419 Hannover (Germany); Knabbe, Ernst-Axel [Deutsches Elektronen-Synchrotron DESY, Notkestrasse 85, D-22607 Hamburg (Germany); Kracht, Dietmar [Laser Zentrum Hannover e.V., Hollerithallee 8, D-30419 Hannover (Germany); Lindner, Axel, E-mail: axel.lindner@desy.d [Deutsches Elektronen-Synchrotron DESY, Notkestrasse 85, D-22607 Hamburg (Germany); List, Jenny [Deutsches Elektronen-Synchrotron DESY, Notkestrasse 85, D-22607 Hamburg (Germany); Meier, Tobias [Max-Planck-Institute for Gravitational Physics, Albert-Einstein-Institute, and Institut fuer Gravitationsphysik, Leibniz Universitaet, Hannover, Callinstrasse 38, D-30167 Hannover (Germany); Meyer, Niels; Notz, Dieter; Redondo, Javier; Ringwald, Andreas [Deutsches Elektronen-Synchrotron DESY, Notkestrasse 85, D-22607 Hamburg (Germany); Wiedemann, Guenter [Hamburger Sternwarte, Gojenbergsweg 112, D-21029 Hamburg (Germany); Willke, Benno [Max-Planck-Institute for Gravitational Physics, Albert-Einstein-Institute, and Institut fuer Gravitationsphysik, Leibniz Universitaet, Hannover, Callinstrasse 38, D-30167 Hannover (Germany)

    2009-12-21

    The ALPS Collaboration runs a 'light shining through a wall' (LSW) experiment to search for photon oscillations into 'weakly interacting sub-eV particles' (WISPs) inside of a superconducting HERA dipole magnet at the site of DESY. In this paper we report on the first successful integration of a large-scale optical resonant cavity to boost the available power for WISP production in this type of experiments. The key elements are a frequency tunable narrow line-width continuous wave laser acting as the primary light source and an electronic feed-back control loop to stabilize the power build-up. We describe and characterize our apparatus and demonstrate the data analysis procedures on the basis of a brief exemplary run.

  7. A data acquisition system for measuring ionization cross section in laser multi-step resonant ionization experiment

    International Nuclear Information System (INIS)

    Qian Dongbin; Guo Yuhui; Zhang Dacheng; Chinese Academy of Sciences, Beijing; Ma Xinwen; Zhao Zhizheng; Wang Yanyu; Zu Kailing

    2006-01-01

    A CAMAC data acquisition system for measuring ionization cross section in laser multi-step resonant ionization experiment is described. The number of scalers in the front-end CAMAC can be adjusted by changing the data read-out table files. Both continuous and manual acquisition models are available, and there is a wide adjustable range from 1 ms to 800 s with the acquisition time unit. The long-term stability, Δt/t, for the data acquisition system with an acquisition time unit of 100 s was measured to be better than ±0.01%, thus validating its reliability in long-term online experimental data acquisition. The time response curves for three electrothermal power-meters were also measured by this DAQ system. (authors)

  8. Structural characterization of phospholipids by matrix-assisted laser desorption/ionization Fourier transform ion cyclotron resonance mass spectrometry.

    Science.gov (United States)

    Marto, J A; White, F M; Seldomridge, S; Marshall, A G

    1995-11-01

    Matrix-assisted laser desorption/ionization (MALDI) Fourier transform ion cyclotron resonance mass spectrometry provides for structural analysis of the principal biological phospholipids: glycerophosphatidylcholine, -ethanolamine, -serine, and -inositol. Both positive and negative molecular or quasimolecular ions are generated in high abundance. Isolated molecular ions may be collisionally activated in the source side of a dual trap mass analyzer, yielding fragments serving to identify the polar head group (positive ion mode) and fatty acid side chains (negative ion mode). Azimuthal quadrupolar excitation following collisionally activated dissociation refocuses productions close to the solenoid axis; subsequent transfer of product ions to the analyzer ion trap allows for high-resolution mass analysis. Cyro-cooling of the sample probe with liquid nitrogen greatly reduces matrix adduction encountered in the negative ion mode.

  9. Using biharmonic laser pumping for preparation of pure and entangled multiexciton states in clusters of resonantly interacting fluorescent centres

    International Nuclear Information System (INIS)

    Basieva, I.T.; Basiev, T.T.; Dietler, G.; Pukhov, K.K.; Sekatskii, S.K.

    2007-01-01

    Use of a biharmonic laser pumping for preparation of pure and entangled multiexciton states in dimers and tetramers of resonantly interacting fluorescent particles is analysed. Special emphasis is given to the preparation of all possible pure exciton states and their maximally entangled Bell states. The general results are illustrated using as an example the pair and quartet centres of neodymium ions in calcium fluoride (M- and N-centres), where all necessary experimental information concerning the interactions and decoherence is available, and experimental preparation of Bell vacuum-single exciton and vacuum-biexciton states has been recently demonstrated. These results can be easily rescaled for the cases of quantum dots and dye molecules. Numerical results are compared with the analytical results obtained for a particular case of the biharmonic excitation of dimers. Excellent agreement between these approaches is demonstrated

  10. Role of Feshbach resonances in enhancing the production of deeply bound ultracold LiRb molecules with laser pulses

    Science.gov (United States)

    Gacesa, Marko; Ghosal, Subhas; Côté, Robin

    2010-03-01

    We investigate the possibility of forming deeply bound LiRb molecules in a two-color photoassociation experiment. Ultracold ^6Li and ^87Rb atoms colliding in the vicinity of a magnetic Feshbach resonance are photoassociated into an excited electronic state. A wavepacket is then formed by exciting a few vibrational levels of the excited state and allowed to propagate. We calculate the time-dependent overlaps between the wave packet and the lowest vibrational levels of the ground state. After the optimal overlap is obtained we use the second laser pulse to dump the wave packet and efficiently populate the deeply bound ro-vibrational levels of ^6Li^87Rb in the ground state. The resulting combination of Feshbach-optimized photoassociation (FOPA) with the time-dependent pump-dump approach will produce a large number of stable ultracold molecules in the ground state. This technique is general and applicable to other systems.

  11. New paradigms for old problems: some (small) advances in laser resonator research at the CSIR

    Science.gov (United States)

    Forbes, Andrew

    2010-02-01

    In this paper we outline new approaches to old problems, namely understanding the transverse modes in Porro prism resonators, and creating methods to select Gaussian beams by phase-only intra-cavity elements. In the process we outline some of the recent research that has taken place within the Mathematical Optics research group.

  12. Fiber Laser Pumped Continuous-wave Singly-resonant Optical Parametric Oscillator

    NARCIS (Netherlands)

    Klein, M.E.; Gross, P.; Walde, T.; Boller, Klaus J.; Auerbach, M.; Wessels, P.; Fallnich, C.; Fejer, Martin M.

    2002-01-01

    We report on the first fiber-pumped CW LiNbO/sub 3/ optical parametric oscillator (OPO). The OPO is singly resonant (SRO) and generates idler wavelengths in the range of 3.0 /spl mu/m to 3.7 /spl mu/m with a maximum output power of 1.9 watt.

  13. Online high sensitivity measurement system for transuranic aerosols

    International Nuclear Information System (INIS)

    Kordas, J.F.; Phelps, P.L.

    1976-01-01

    A measurement system for transuranic aerosols has been designed that will be able to withstand the corrosive nature of stack effluents and yet have extremely high sensitivity. It will be capable of measuring 1 maximum permissible concentration (MPC) of plutonium or americium in 30 minutes with a fractional standard deviation of less than 0.33. Background resulting from 218 Po is eliminated by alpha energy discrimination and a decay scheme analysis. A microprocessor controls all data acquisition, data reduction, and instrument calibration

  14. Magnetic resonance imaging-guided focused laser interstitial thermal therapy for subinsular metastatic adenocarcinoma: technical case report.

    Science.gov (United States)

    Hawasli, Ammar H; Ray, Wilson Z; Murphy, Rory K J; Dacey, Ralph G; Leuthardt, Eric C

    2012-06-01

    To describe the novel use of the AutoLITT System (Monteris Medical, Winnipeg, Manitoba, Canada) for focused laser interstitial thermal therapy (LITT) with intraoperative magnetic resonance imaging (MRI) and stereotactic image guidance for the treatment of metastatic adenocarcinoma in the left insula. The patient was a 61-year-old right-handed man with a history of metastatic adenocarcinoma of the colon. He had previously undergone resection of multiple lesions, Gamma Knife radiosurgery, and whole-brain radiation. Despite treatment of a left insular tumor, serial imaging revealed that the lesion continued to enlarge. Given the refractory nature of this tumor to radiation and the deep-seated location, the patient elected to undergo LITT treatment. The center of the lesion and entry point on the scalp were identified with STEALTH (Medtronic, Memphis, Tennessee) image-guided navigation. The AXiiiS Stereotactic Miniframe (Monteris Medical) for the LITT system was secured onto the skull, and a trajectory was defined to achieve access to the centroid of the tumor. After a burr hole was made, a gadolinium template probe was inserted into the AXiiiS base. The trajectory was confirmed via an intraoperative MRI, and the LITT probe driver was attached to the base and CO2-cooled, side-firing laser LITT probe. The laser was activated and thermometry images were obtained. Two trajectories, posteromedial and anterolateral, produced satisfactory tumor ablation. LITT with intraoperative MRI and stereotactic image guidance is a newly available, minimally invasive, and therapeutically viable technique for the treatment of deep seated brain tumors.

  15. Intensity and pressure dependence of resonance fluorescence of OH induced by a tunable UV laser

    Science.gov (United States)

    Killinger, D. K.; Wang, C. C.; Hanabusa, M.

    1976-01-01

    The intensity and pressure dependence of the fluorescence spectrum of OH in the presence of N2 and H2O molecules was studied. Saturation of the absorption transition was observed at low pressures, and the corresponding fluorescence signal was found to vary as the square root of the exciting intensity. This observed dependence agreed with the predicted dependence which took into account the presence of laser modes in the spectrum of the exciting radiation. With full laser power incident, a saturation parameter as high as 3 x 10 to the 5th was observed. The fluorescence spectrum was found to peak at 3145 and at 3090 A, with the relative peak intensities dependent upon gas pressures and upon the particular rotational electronic transition used for excitation. It is concluded that vibrational relaxation of the electronically excited OH due to water vapor in the system plays a dominant role in determining the observed fluorescence spectrum.

  16. Laser heating tunability by off-resonant irradiation of gold nanoparticles.

    Science.gov (United States)

    Hormeño, Silvia; Gregorio-Godoy, Paula; Pérez-Juste, Jorge; Liz-Marzán, Luis M; Juárez, Beatriz H; Arias-Gonzalez, J Ricardo

    2014-01-29

    Temperature changes in the vicinity of a single absorptive nanostructure caused by local heating have strong implications in technologies such as integrated electronics or biomedicine. Herein, the temperature changes in the vicinity of a single optically trapped spherical Au nanoparticle encapsulated in a thermo-responsive poly(N-isopropylacrylamide) shell (Au@pNIPAM) are studied in detail. Individual beads are trapped in a counter-propagating optical tweezers setup at various laser powers, which allows the overall particle size to be tuned through the phase transition of the thermo-responsive shell. The experimentally obtained sizes measured at different irradiation powers are compared with average size values obtained by dynamic light scattering (DLS) from an ensemble of beads at different temperatures. The size range and the tendency to shrink upon increasing the laser power in the optical trap or by increasing the temperature for DLS agree with reasonable accuracy for both approaches. Discrepancies are evaluated by means of simple models accounting for variations in the thermal conductivity of the polymer, the viscosity of the aqueous solution and the absorption cross section of the coated Au nanoparticle. These results show that these parameters must be taken into account when considering local laser heating experiments in aqueous solution at the nanoscale. Analysis of the stability of the Au@pNIPAM particles in the trap is also theoretically carried out for different particle sizes. © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  17. Laser-optogalvanic studies of the 4p5 ns and nd autoionizing resonances in krypton

    International Nuclear Information System (INIS)

    Baig, M A; Hanif, M; Aslam, M

    2008-01-01

    We report new measurements of the odd-parity autoionizing resonances in krypton using resonant two-photon excitation from the 4p 5 5s[3/2] 2 metastable level in a mild DC discharge and an optogalvanic detection technique. We have observed the 4p 5 ns [1/2] 0,1 , 4p 5 nd [3/2] 2 and 4p 5 nd [5/2] 2,3 autoionizing resonances excited from three intermediate levels 4p 5 5p' [1/2] 1 , 4p 5 5p' [3/2] 1 and 4p 5 5p' [3/2] 2 . The spectra are notable for the absence of the broad autoionizing 4p 5 nd [3/2] 1 series which dominates in the photo-absorption spectrum from the ground state. The prominent transitions follow ΔK = ΔJ = Δl selection rules of the JK-coupling scheme. We report nearly 100 new energy levels in krypton besides the quantum defects and the reduced widths Γ r Γ(ν) 3 of the nd' [3/2] 2 , nd' [5/2] 2 and nd' [5/2] 3 Rydberg states

  18. Polymer laser bio-sensors

    DEFF Research Database (Denmark)

    Kristensen, Anders; Vannahme, Christoph; Hermannsson, Pétur Gordon

    2014-01-01

    Organic dye based distributed feed-back lasers, featuring narrow linewidth and thus high quality spectral resolution, are used as highly sensitive refractive index sensors. The design, fabrication and application of the laser intra-cavity sensors are discussed....

  19. The investigations of nanoclusters and micron-sized periodic structures created at the surface of the crystal and amorphous silica by resonant CO2 laser irradiation

    Directory of Open Access Journals (Sweden)

    Mukhamedgalieva A.F.

    2017-01-01

    Full Text Available The creation of nanoclasters and micrometer sized periodical structures at the surface of silica (crystal quartz and fused quartz by action of pulsed CO2 laser radiation (pulse energy of 1 J, pulse time of 70 ns have been investigated. The laser action on the surface of samples lead to appearance of two kind of structures – periodical micron-sized structures with the period length close to wave length of CO2 laser irradiation and nanoclusters with size close to 50-100 nanometers. This creation connects with the intensive ablation of matter at the maxima of standing waves which are a results of the interference of falling and surfaces waves. This connects with the resonant absorption of infrared laser radiation by silicate minerals.

  20. A highly sensitive and specific assay for vertebrate collagenase

    International Nuclear Information System (INIS)

    Sodek, J.; Hurum, S.; Feng, J.

    1981-01-01

    A highly sensitive and specific assay for vertebrate collagenase has been developed using a [ 14 C]-labeled collagen substrate and a combination of SDS-PAGE (sodium dodecyl sulfate-polyacrylamide gel electrophoresis) and fluorography to identify and quantitate the digestion products. The assay was sufficiently sensitive to permit the detection and quantitation of collagenase activity in 0.1 μl of gingival sulcal fluid, and in samples of cell culture medium without prior concentration. The assay has also been used to detect the presence of inhibitors of collagenolytic enzymes in various cell culture fluids. (author)

  1. Highly Sensitive Flexible Magnetic Sensor Based on Anisotropic Magnetoresistance Effect.

    Science.gov (United States)

    Wang, Zhiguang; Wang, Xinjun; Li, Menghui; Gao, Yuan; Hu, Zhongqiang; Nan, Tianxiang; Liang, Xianfeng; Chen, Huaihao; Yang, Jia; Cash, Syd; Sun, Nian-Xiang

    2016-11-01

    A highly sensitive flexible magnetic sensor based on the anisotropic magnetoresistance effect is fabricated. A limit of detection of 150 nT is observed and excellent deformation stability is achieved after wrapping of the flexible sensor, with bending radii down to 5 mm. The flexible AMR sensor is used to read a magnetic pattern with a thickness of 10 μm that is formed by ferrite magnetic inks. © 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  2. High sensitivity on-line monitor for radioactive effluent

    Energy Technology Data Exchange (ETDEWEB)

    Sasaki, Toshimi [Tohoku Electric Power Co. Ltd., Sendai (Japan); Ishizuka, Akira; Abe, Eisuke; Inoue, Yasuhiko; Fujii, Masaaki; Kitaguchi, Hiroshi; Doi, Akira

    1983-04-01

    A new approach for a highly sensitive effluent monitor is presented. The free flow type monitor, which consists of a straightener, nozzle, monitoring section and ..gamma..-ray detector, is demonstrated to be effective in providing long term stability. The 160 start-and-stop cycles of effluent discharge were repeated in a 120-h testing period. Results showed a background increase was not observed for the free flow type monitor. The background count rate was calibrated to the lowest detection limit to be 2.2 x 10/sup -2/ Bq/ml for a 300 s measurement time.

  3. Resonant parametric interference effect in spontaneous bremsstrahlung of an electron in the field of a nucleus and two pulsed laser waves

    Science.gov (United States)

    Lebed', A. A.; Padusenko, E. A.; Roshchupkin, S. P.; Dubov, V. V.

    2018-04-01

    Electron-nucleus bremsstrahlung in the field of two moderately strong pulsed laser waves in the case of incommensurate frequencies is theoretically studied under resonant conditions. The process is studied in detail in a special kinematic region, where stimulated processes with correlated emission and absorption of photons of the first and second waves become predominant (parametric interference effect). The availability of this region is caused by interference of the first and second laser waves. The correspondence between the emission angle and the final-electron energy is established in this interference kinematic. In this case, the cross-sectional properties are determined by the multiphoton quantum interference parameter, which is proportional to the product of intensities of the first and second waves. The resonant differential cross section of electron-nucleus spontaneous bremsstrahlung with simultaneous registration of both emission angles of the spontaneous photon and the scattered electron can exceed by four or five orders of magnitude the corresponding cross section in the absence of an external field. It was shown for nonrelativistic electrons that the resonant cross section of the studied process in the field of two pulsed laser waves within the interference region in two order of magnitude may exceed corresponding cross sections at other scattering kinematics. The obtained results may be experimentally verified, for example, by scientific facilities at sources of pulsed laser radiation (such as SLAC, FAIR, XFEL, ELI).

  4. Observation of the nearly diurnal resonance of the earth using a laser strainmeter

    Science.gov (United States)

    Levine, J.

    1978-01-01

    The response of the Earth to the diurnal and semidiurnal tidal excitations was studied. Results show that there is significant structure in the response of the earth to tidal excitations near one cycle/sidereal day. This structure agrees with the resonance behavior predicted from the calculations of the forced elasticgravitational response of an elliptical, rotating earth with a liquid outer core. The data is used to test for possible preferred frames and spatial anisotropies. Upper bounds on the parameterized post-Newtonian (PPN) parameters were examined.

  5. Theory of resonant multiphoton ionization of krypton by intense ultraviolet laser radiation

    International Nuclear Information System (INIS)

    Tang, X.; Lambropoulos, P.; L'Huillier, A.; Dixit, S.N.

    1989-01-01

    We present a theoretical interpretation of the experimental results on three-photon-resonant four-photon ionization of Kr reported by Landen, Perry, and Campbell [Phys. Rev. Lett. 59, 2558 (1987)] and Perry and Landen [Phys. Rev. A 38, 2815 (1988)]. Our calculations are based on multichannel quantum-defect theory combined with a density-matrix formalism describing the spatiotemporal development of the process. We obtain good agreement with the data, which even at intensities as high as 10 14 W/cm 2 show the imprint of the underlying atomic structure

  6. Generation of auroral hectometer radio emission at the laser cyclotron resonance (ωp≥ωH)

    International Nuclear Information System (INIS)

    Vlasov, V.G.

    1992-01-01

    Generation of auroral hectometer (AHR) and kilometer (AKR) radio emission at a maser cyclotron resonance (MCR) in a relatively dense plasma (ω p ≥ω H ) is theoretically studied. The conclusion is made that availability of two-dimensional small-scale inhomogeneity of plasma density is the basic condition for the AHR generation at the MCR by auroral electron beams. The small-scale inhomogeneity of the auroral plasma, measured on satelites, meets by its parameters the conditions for the generation of auroral radio emission

  7. Highly sensitive detection of urinary cadmium to assess personal exposure

    Energy Technology Data Exchange (ETDEWEB)

    Argun, Avni A.; Banks, Ashley M.; Merlen, Gwendolynne; Tempelman, Linda A. [Giner, Inc., 89 Rumford Ave., Newton 02466, MA United States (United States); Becker, Michael F.; Schuelke, Thomas [Fraunhofer USA – CCL, 1449 Engineering Research Ct., East Lansing 48824, MI (United States); Dweik, Badawi M., E-mail: bdweik@ginerinc.com [Giner, Inc., 89 Rumford Ave., Newton 02466, MA United States (United States)

    2013-04-22

    Highlights: ► An electrochemical sensor capable of detecting cadmium at parts-per-billion levels in urine. ► A novel fabrication method for Boron-Doped Diamond (BDD) ultramicroelectrode (UME) arrays. ► Unique combination of BDD UME arrays and a differential pulse voltammetry algorithm. ► High sensitivity, high reproducibility, and very low noise levels. ► Opportunity for portable operation to assess on-site personal exposure. -- Abstract: A series of Boron-Doped Diamond (BDD) ultramicroelectrode arrays were fabricated and investigated for their performance as electrochemical sensors to detect trace level metals such as cadmium. The steady-state diffusion behavior of these sensors was validated using cyclic voltammetry followed by electrochemical detection of cadmium in water and in human urine to demonstrate high sensitivity (>200 μA ppb{sup −1} cm{sup −2}) and low background current (<4 nA). When an array of ultramicroelectrodes was positioned with optimal spacing, these BDD sensors showed a sigmoidal diffusion behavior. They also demonstrated high accuracy with linear dose dependence for quantification of cadmium in a certified reference river water sample from the U.S. National Institute of Standards and Technology (NIST) as well as in a human urine sample spiked with 0.25–1 ppb cadmium.

  8. Towards highly sensitive strain sensing based on nanostructured materials

    International Nuclear Information System (INIS)

    Dao, Dzung Viet; Nakamura, Koichi; Sugiyama, Susumu; Bui, Tung Thanh; Dau, Van Thanh; Yamada, Takeo; Hata, Kenji

    2010-01-01

    This paper presents our recent theoretical and experimental study of piezo-effects in nanostructured materials for highly sensitive, high resolution mechanical sensors. The piezo-effects presented here include the piezoresistive effect in a silicon nanowire (SiNW) and single wall carbon nanotube (SWCNT) thin film, as well as the piezo-optic effect in a Si photonic crystal (PhC) nanocavity. Firstly, the electronic energy band structure of the silicon nanostructure is discussed and simulated by using the First-Principles Calculations method. The result showed a remarkably different energy band structure compared with that of bulk silicon. This difference in the electronic state will result in different physical, chemical, and therefore, sensing properties of silicon nanostructures. The piezoresistive effects of SiNW and SWCNT thin film were investigated experimentally. We found that, when the width of ( 110 ) p-type SiNW decreases from 500 to 35 nm, the piezoresistive effect increases by more than 60%. The longitudinal piezoresistive coefficient of SWCNT thin film was measured to be twice that of bulk p-type silicon. Finally, theoretical investigations of the piezo-optic effect in a PhC nanocavity based on Finite Difference Time Domain (FDTD) showed extremely high resolution strain sensing. These nanostructures were fabricated based on top-down nanofabrication technology. The achievements of this work are significant for highly sensitive, high resolution and miniaturized mechanical sensors

  9. Design of highly sensitive multichannel bimetallic photonic crystal fiber biosensor

    Science.gov (United States)

    Hameed, Mohamed Farhat O.; Alrayk, Yassmin K. A.; Shaalan, Abdelhamid A.; El Deeb, Walid S.; Obayya, Salah S. A.

    2016-10-01

    A design of a highly sensitive multichannel biosensor based on photonic crystal fiber is proposed and analyzed. The suggested design has a silver layer as a plasmonic material coated by a gold layer to protect silver oxidation. The reported sensor is based on detection using the quasi transverse electric (TE) and quasi transverse magnetic (TM) modes, which offers the possibility of multichannel/multianalyte sensing. The numerical results are obtained using a finite element method with perfect matched layer boundary conditions. The sensor geometrical parameters are optimized to achieve high sensitivity for the two polarized modes. High-refractive index sensitivity of about 4750 nm/RIU (refractive index unit) and 4300 nm/RIU with corresponding resolutions of 2.1×10-5 RIU, and 2.33×10-5 RIU can be obtained according to the quasi TM and quasi TE modes of the proposed sensor, respectively. Further, the reported design can be used as a self-calibration biosensor within an unknown analyte refractive index ranging from 1.33 to 1.35 with high linearity and high accuracy. Moreover, the suggested biosensor has advantages in terms of compactness and better integration of microfluidics setup, waveguide, and metallic layers into a single structure.

  10. Measurement system for high-sensitivity LIBS analysis using ICCD camera in LabVIEW environment

    International Nuclear Information System (INIS)

    Zaytsev, S M; Popov, A M; Zorov, N B; Labutin, T A

    2014-01-01

    A measurement system based on ultrafast (up to 10 ns time resolution) intensified CCD detector ''Nanogate-2V'' (Nanoscan, Russia) was developed for high-sensitivity analysis by Laser-Induced Breakdown Spectrometry (LIBS). LabVIEW environment provided a high level of compatibility with variety of electronic instruments and an easy development of user interface, while Visual Studio environment was used for creation of LabVIEW compatible dll library with the use of ''Nanogate-2V'' SDK. The program for camera management and laser-induced plasma spectra registration was created with the use of Call Library Node in LabVIEW. An algorithm of integration of the second device ADC ''PCI-9812'' (ADLINK) to the measurement system was proposed and successfully implemented. This allowed simultaneous registration of emission and acoustic signals under laser ablation. The measured resolving power of spectrometer-ICCD system was equal to 12000 at 632 nm. An electron density of laser plasma was estimated with the use of H-α Balmer line. Steel spectra obtained at different delays were used for selection of the optimal conditions for manganese analytical signal registration. The feature of accumulation of spectra from several laser pulses was shown. The accumulation allowed reliable observation of silver signal at 328.07 nm in the LIBS spectra of soil (C Ag = 4.5 ppm). Finally, the correlation between acoustic and emission signals of plasma was found. Thus, technical possibilities of the developed LIBS system were demonstrated both for plasma diagnostics and analytical measurements

  11. Mode-locking peculiarities in an all-fiber erbium-doped ring ultrashort pulse laser with a highly-nonlinear resonator

    Science.gov (United States)

    Dvoretskiy, Dmitriy A.; Sazonkin, Stanislav G.; Kudelin, Igor S.; Orekhov, Ilya O.; Pnev, Alexey B.; Karasik, Valeriy E.; Denisov, Lev K.

    2017-12-01

    Today ultrashort pulse (USP) fiber lasers are in great demand in a frequency metrology field, THz pulse spectroscopy, optical communication, quantum optics application, etc. Therefore mode-locked (ML) fiber lasers have been extensively investigated over the last decade due the number of scientific, medical and industrial applications. It should be noted, that USP fiber lasers can be treated as an ideal platform to expand future applications due to the complex ML nonlinear dynamics in a laser resonator. Up to now a series of novel ML regimes have been investigated e.g. self-similar pulses, noise-like pulses, multi-bound solitons and soliton rain generation. Recently, we have used a highly nonlinear germanosilicate fiber (with germanium oxides concentration in the core 50 mol. %) inside the resonator for more reliable and robust launching of passive mode-locking based on the nonlinear polarization evolution effect in fibers. In this work we have measured promising and stable ML regimes such as stretched pulses, soliton rain and multi-bound solitons formed in a highly-nonlinear ring laser and obtained by intracavity group velocity dispersion (GVD) variation in slightly negative region. As a result, we have obtained the low noise ultrashort pulse generation with duration 59 dB) and relative intensity noise <-101 dBc / Hz.

  12. A single-longitudinal-mode Brillouin fiber laser passively stabilized at the pump resonance frequency with a dynamic population inversion grating

    International Nuclear Information System (INIS)

    Spirin, V V; López-Mercado, C A; Kinet, D; Mégret, P; Fotiadi, A A; Zolotovskiy, I O

    2013-01-01

    We demonstrate a single-longitudinal-mode Brillouin ring fiber laser passively stabilized at the resonance frequency with a 1.7 m section that is an unpumped polarization-maintaining erbium-doped fiber. The two coupled all-fiber Fabry–Perot interferometers that comprise the cavity, in combination with the dynamical population inversion gratings self-induced in the active fiber, provide adaptive pump-mode selection and Stokes wave generation at the same time. The laser is shown to emit a single-frequency Stokes wave with a linewidth narrower than 100 Hz. (letter)

  13. A virus-MIPs fluorescent sensor based on FRET for highly sensitive detection of JEV.

    Science.gov (United States)

    Liang, Caishuang; Wang, Huan; He, Kui; Chen, Chunyan; Chen, Xiaoming; Gong, Hang; Cai, Changqun

    2016-11-01

    Major stumbling blocks in the recognition and detection of virus are the unstable biological recognition element or the complex detection means. Here a fluorescent sensor based on virus-molecular imprinted polymers (virus-MIPs) was designed for specific recognition and highly sensitive detection of Japanese encephalitis virus (JEV). The virus-MIPs were anchored on the surface of silica microspheres modified by fluorescent dye, pyrene-1-carboxaldehyde (PC). The fluorescence intensity of PC can be enhanced by the principle of fluorescence resonance energy transfer (FRET), where virus acted as energy donor and PC acted as energy acceptor. The enhanced fluorescence intensity was proportional to the concentration of virus in the range of 24-960pM, with a limit of detection (LOD, 3σ) of 9.6pM, and the relative standard deviation was 1.99%. In additional, the specificity study confirmed the resultant MIPs has high-selectivity for JEV. This sensor would become a new key for the detection of virus because of its high sensitive, simple operation, high stability and low cost. Copyright © 2016. Published by Elsevier B.V.

  14. Resonant third harmonic generation of KrF laser in Ar gas

    Energy Technology Data Exchange (ETDEWEB)

    Rakowski, R. [Department of Experimental Physics, University of Szeged, 6720 Szeged, Dóm tér 9 (Hungary); Institute of Optoelectronics, Military University of Technology, Gen. S. Kaliskiego 2, 00–908 Warsaw (Poland); Barna, A. [Department of Experimental Physics, University of Szeged, 6720 Szeged, Dóm tér 9 (Hungary); Wigner Research Centre for Physics, Institute for Particle and Nuclear Physics, EURATOM Association HAS, 1121 Budapest, XII. Konkoly Thege Miklós út 29-33 (Hungary); Suta, T.; Földes, I. B. [Wigner Research Centre for Physics, Institute for Particle and Nuclear Physics, EURATOM Association HAS, 1121 Budapest, XII. Konkoly Thege Miklós út 29-33 (Hungary); Bohus, J.; Szatmári, S. [Department of Experimental Physics, University of Szeged, 6720 Szeged, Dóm tér 9 (Hungary); Mikołajczyk, J.; Bartnik, A.; Fiedorowicz, H. [Institute of Optoelectronics, Military University of Technology, Gen. S. Kaliskiego 2, 00–908 Warsaw (Poland); Verona, C. [Department of Mechanical Engineering, University “Tor Vergata”, Via Orazio Raimondo, 18–00173, Rome (Italy); Verona Rinati, G. [Department of Industrial Engineering, University “Tor Vergata”, Via Orazio Raimondo, 18–00173, Rome (Italy); Margarone, D. [Institute of Physics ASCR, v.v.i. (FZU), ELI-Beamlines Project, 182 21 Prague (Czech Republic); Nowak, T. [Institute of Nuclear Physics, PAN, E. Radzikowskiego 152, 31–342 Cracow (Poland); and others

    2014-12-15

    Investigations of emission of harmonics from argon gas jet irradiated by 700 fs, 5 mJ pulses from a KrF laser are presented. Harmonics conversion was optimized by varying the experimental geometry and the nozzle size. For the collection of the harmonic radiation silicon and solar-blind diamond semiconductor detectors equipped with charge preamplifiers were applied. The possibility of using a single-crystal CVD diamond detector for separate measurement of the 3rd harmonic in the presence of a strong pumping radiation was explored. Our experiments show that the earlier suggested 0.7% conversion efficiency can really be obtained, but only in the case when phase matching is optimized with an elongated gas target length corresponding to the length of coherence.

  15. Resonant laser power build-up in ALPS. A 'light-shining-through-walls' experiment

    International Nuclear Information System (INIS)

    Ehret, Klaus; Ghazaryan, Samvel; Frede, Maik

    2009-05-01

    The ALPS collaboration runs a light-shining-through-walls (LSW) experiment to search for photon oscillations into weakly interacting sub-eV particles (WISPs) inside of a superconducting HERA dipole magnet at the site of DESY. In this paper we report on the first successful integration of a large-scale optical cavity to boost the available power for WISP production in this type of experiments. The key elements are a frequency tunable narrow line-width continuous wave laser acting as the primary light source and an electronic feed-back control loop to stabilize the power build-up. We describe and characterize our apparatus and demonstrate the data analysis procedures on the basis of a brief exemplary run. (orig.)

  16. Line overlap measurements for resonant photo-pumping of x-ray lasers

    International Nuclear Information System (INIS)

    Elliott, S.R.; Beiersdorfer, P.; Nilsen, J.

    1993-01-01

    Measurement taken on the LLNL EBIT to search for the possible photo-pumping of the 3p-3s lasing transitions in Ni-like ions of elements with Z=30--40 and the 4d-4p lasing transitions in Ne-like ions of elements with Z=47-73 are reported. A high-resolution crystral spectrometer was used to measure wavelengths of the Ne-like 2p-4d and the Ni-like 3d-5f and 3d-6f laser level feeding transitions relative to candidate pump lines in various H-, He-, and Ni-like ions. To date, the most promising candidate is Ni-like Pt pumping Ne-like Rb at 2512 eV. The line energies differ by 0.4±0.1 eV or by 160 ppm

  17. Application of the laser induced fluorescence to the investigation of highly magnetized plasmas, heated by ion cyclotron resonance

    International Nuclear Information System (INIS)

    Pailloux, A.

    1997-01-01

    This work has been achieved in the frame of isotopic separation studies by in cyclotron resonance. For this purpose, in a highly magnetized (2 to 3 Tesla) and non-collisional (10 12 ions/cm 3 ) plasma, composed of metallic ions, a wave near the ion cyclotron frequency is thrown in order to heat selectively a given species. A laser induced fluorescence (LIP) has been developed on barium and gadolinium plasmas. The Larmor gyration of ions greatly modifies the interaction, which has been modelled through the time-dependent Schroedinger equation. The obtained excitation probably has been integrated over all the ions excited in the measurement volume in order to check that the LIF still leads to the distribution function of ion velocities. The influence of the Larmor motion of ions on the spectral distribution of LIF has been derived both theoretically and experimentally. The LIF diagnostics has been achieved with a dye O'ring laser. The barium ion has been excited on the transition 6142 angstrom, using rhodamine 6G dye, and the gadolinium ion on the pseudo-triplet 3861 angstrom, using exalite dye. Data treatment has been developed taking into account the Zeeman effect and the different heating of isotopes. The ionic temperature (from 1 eV to some hundreds eV) has been measured as a function of radiofrequency heating. Our experimental results are in good agreement with the selective heating theory. Also, the ion velocity distribution function has been found locally Maxwellian. And the behaviour of the plasma has been studied as a function of control parameters of the plasma source. (author)

  18. High-speed asynchronous optical sampling for high-sensitivity detection of coherent phonons

    International Nuclear Information System (INIS)

    Dekorsy, T; Taubert, R; Hudert, F; Schrenk, G; Bartels, A; Cerna, R; Kotaidis, V; Plech, A; Koehler, K; Schmitz, J; Wagner, J

    2007-01-01

    A new optical pump-probe technique is implemented for the investigation of coherent acoustic phonon dynamics in the GHz to THz frequency range which is based on two asynchronously linked femtosecond lasers. Asynchronous optical sampling (ASOPS) provides the performance of on all-optical oscilloscope and allows us to record optically induced lattice dynamics over nanosecond times with femtosecond resolution at scan rates of 10 kHz without any moving part in the set-up. Within 1 minute of data acquisition time signal-to-noise ratios better than 10 7 are achieved. We present examples of the high-sensitivity detection of coherent phonons in superlattices and of the coherent acoustic vibration of metallic nanoparticles

  19. Ultra slow muon microscopy by laser resonant ionization at J-PARC, MUSE

    Energy Technology Data Exchange (ETDEWEB)

    Miyake, Y., E-mail: yasuhiro.miyake@kek.jp; Ikedo, Y.; Shimomura, K.; Strasser, P.; Kawamura, N.; Nishiyama, K.; Koda, A.; Fujimori, H.; Makimura, S.; Nakamura, J.; Nagatomo, T.; Kadono, R. [High Energy Accelerator Research Organization (KEK), Muon Science Laboratory (Japan); Torikai, E. [Yamanashi University, Faculty of Engineering (Japan); Iwasaki, M. [RIKEN Nishina Center, Advanced Meson Science Laboratory (Japan); Wada, S.; Saito, N. [RIKEN, Advanced Science Institute (Japan); Okamura, K. [RIKEN-WAKO Incubation Plaza 301, Megaopto Co., Ltd. (Japan); Yokoyama, K. [RIKEN Nishina Center, Advanced Meson Science Laboratory (Japan); Ito, T.; Higemoto, W. [J-PARC Center, Muon Section, Materials and Life Science Division (Japan)

    2013-04-15

    As one of the principal muon beam line at the J-PARC muon facility (MUSE), we are now constructing a Muon beam line (U-Line), which consists of a large acceptance solenoid made of mineral insulation cables (MIC), a superconducting curved transport solenoid and superconducting axial focusing magnets. There, we can extract 2 Multiplication-Sign 10{sup 8}/s surface muons towards a hot tungsten target. At the U-Line, we are now establishing a new type of muon microscopy; a new technique with use of the intense ultra-slow muon source generated by resonant ionization of thermal Muonium (designated as Mu; consisting of a {mu}{sup + } and an e{sup - }) atoms generated from the surface of the tungsten target. In this contribution, the latest status of the Ultra Slow Muon Microscopy project, fully funded, is reported.

  20. Ultra slow muon microscopy by laser resonant ionization at J-PARC, MUSE

    Science.gov (United States)

    Miyake, Y.; Ikedo, Y.; Shimomura, K.; Strasser, P.; Kawamura, N.; Nishiyama, K.; Koda, A.; Fujimori, H.; Makimura, S.; Nakamura, J.; Nagatomo, T.; Kadono, R.; Torikai, E.; Iwasaki, M.; Wada, S.; Saito, N.; Okamura, K.; Yokoyama, K.; Ito, T.; Higemoto, W.

    2013-04-01

    As one of the principal muon beam line at the J-PARC muon facility (MUSE), we are now constructing a Muon beam line (U-Line), which consists of a large acceptance solenoid made of mineral insulation cables (MIC), a superconducting curved transport solenoid and superconducting axial focusing magnets. There, we can extract 2 × 108/s surface muons towards a hot tungsten target. At the U-Line, we are now establishing a new type of muon microscopy; a new technique with use of the intense ultra-slow muon source generated by resonant ionization of thermal Muonium (designated as Mu; consisting of a μ + and an e - ) atoms generated from the surface of the tungsten target. In this contribution, the latest status of the Ultra Slow Muon Microscopy project, fully funded, is reported.

  1. Design of a Piezoelectric Accelerometer with High Sensitivity and Low Transverse Effect

    Directory of Open Access Journals (Sweden)

    Bian Tian

    2016-09-01

    Full Text Available In order to meet the requirements of cable fault detection, a new structure of piezoelectric accelerometer was designed and analyzed in detail. The structure was composed of a seismic mass, two sensitive beams, and two added beams. Then, simulations including the maximum stress, natural frequency, and output voltage were carried out. Moreover, comparisons with traditional structures of piezoelectric accelerometer were made. To verify which vibration mode is the dominant one on the acceleration and the space between the mass and glass, mode analysis and deflection analysis were carried out. Fabricated on an n-type single crystal silicon wafer, the sensor chips were wire-bonged to printed circuit boards (PCBs and simply packaged for experiments. Finally, a vibration test was conducted. The results show that the proposed piezoelectric accelerometer has high sensitivity, low resonance frequency, and low transverse effect.

  2. A high sensitivity momentum flux measuring instrument for plasma thruster exhausts and diffusive plasmas.

    Science.gov (United States)

    West, Michael D; Charles, Christine; Boswell, Rod W

    2009-05-01

    A high sensitivity momentum flux measuring instrument based on a compound pendulum has been developed for use with electric propulsion devices and radio frequency driven plasmas. A laser displacement system, which builds upon techniques used by the materials science community for surface stress measurements, is used to measure with high sensitivity the displacement of a target plate placed in a plasma thruster exhaust. The instrument has been installed inside a vacuum chamber and calibrated via two different methods and is able to measure forces in the range of 0.02-0.5 mN with a resolution of 15 microN. Measurements have been made of the force produced from the cold gas flow and with a discharge ignited using argon propellant. The plasma is generated using a Helicon Double Layer Thruster prototype. The instrument target is placed about 1 mean free path for ion-neutral charge exchange collisions downstream of the thruster exit. At this position, the plasma consists of a low density ion beam (10%) and a much larger downstream component (90%). The results are in good agreement with those determined from the plasma parameters measured with diagnostic probes. Measurements at various flow rates show that variations in ion beam velocity and plasma density and the resulting momentum flux can be measured with this instrument. The instrument target is a simple, low cost device, and since the laser displacement system used is located outside the vacuum chamber, the measurement technique is free from radio frequency interference and thermal effects. It could be used to measure the thrust in the exhaust of other electric propulsion devices and the momentum flux of ion beams formed by expanding plasmas or fusion experiments.

  3. Development of high sensitivity and high speed large size blank inspection system LBIS

    Science.gov (United States)

    Ohara, Shinobu; Yoshida, Akinori; Hirai, Mitsuo; Kato, Takenori; Moriizumi, Koichi; Kusunose, Haruhiko

    2017-07-01

    The production of high-resolution flat panel displays (FPDs) for mobile phones today requires the use of high-quality large-size photomasks (LSPMs). Organic light emitting diode (OLED) displays use several transistors on each pixel for precise current control and, as such, the mask patterns for OLED displays are denser and finer than the patterns for the previous generation displays throughout the entire mask surface. It is therefore strongly demanded that mask patterns be produced with high fidelity and free of defect. To enable the production of a high quality LSPM in a short lead time, the manufacturers need a high-sensitivity high-speed mask blank inspection system that meets the requirement of advanced LSPMs. Lasertec has developed a large-size blank inspection system called LBIS, which achieves high sensitivity based on a laser-scattering technique. LBIS employs a high power laser as its inspection light source. LBIS's delivery optics, including a scanner and F-Theta scan lens, focus the light from the source linearly on the surface of the blank. Its specially-designed optics collect the light scattered by particles and defects generated during the manufacturing process, such as scratches, on the surface and guide it to photo multiplier tubes (PMTs) with high efficiency. Multiple PMTs are used on LBIS for the stable detection of scattered light, which may be distributed at various angles due to irregular shapes of defects. LBIS captures 0.3mμ PSL at a detection rate of over 99.5% with uniform sensitivity. Its inspection time is 20 minutes for a G8 blank and 35 minutes for G10. The differential interference contrast (DIC) microscope on the inspection head of LBIS captures high-contrast review images after inspection. The images are classified automatically.

  4. Probing ultrafast changes of spin and charge density profiles with resonant XUV magnetic reflectivity at the free-electron laser FERMI

    Directory of Open Access Journals (Sweden)

    C. Gutt

    2017-09-01

    Full Text Available We report the results of resonant magnetic XUV reflectivity experiments performed at the XUV free-electron laser FERMI. Circularly polarized XUV light with the photon energy tuned to the Fe M2,3 edge is used to measure resonant magnetic reflectivities and the corresponding Q-resolved asymmetry of a Permalloy/Ta/Permalloy trilayer film. The asymmetry exhibits ultrafast changes on 240 fs time scales upon pumping with ultrashort IR laser pulses. Depending on the value of the wavevector transfer Qz, we observe both decreasing and increasing values of the asymmetry parameter, which is attributed to ultrafast changes in the vertical spin and charge density profiles of the trilayer film.

  5. Development of an underwater high sensitivity Cherenkov detector: Sea Urchin

    International Nuclear Information System (INIS)

    Camerini, U.; McGibney, D.; Roberts, A.

    1982-01-01

    The need for a high gain, high sensitivity Cherenkov light sensor to be used in a deep underwater muon and neutrino detector (DUMAND) array has led to the design of the Sea Urchin detector. In this design a spherical photocathode PMTis optically coupled through a glass hemisphere to a large number of glass spines, each of which is filled with a wavelength-shifting (WLS) solution of a high quantum efficiency phosphor. The Cherenkov radiation is absorbed in the spine, isotropically re-radiated at a longer wavelength, and a fraction of the fluorescent light is internally reflected in the spine, and guided to the photomultiplier concentrically located in the glass hemisphere. Experiments measuring the optical characteristics of the spines and computer programs simulating light transformation and detection cross sections are described. Overall optical gains in the range 5-10 are achieved. The WLS solution is inexpensive, and may have other applications. (orig.)

  6. High sensitivity tests of the standard model for electroweak interactions

    International Nuclear Information System (INIS)

    Koetke, D.D.

    1992-01-01

    The work done on this project was focussed mainly on LAMPF experiment E969 known as the MEGA experiment, a high sensitivity search for the lepton family number violating decay μ → eγ to a sensitivity which, measured in terms of the branching ratio, BR = [μ→eγ]/[μ→e ν μ ν e ] ∼10 -13 is over two orders of magnitude better than previously reported values. The work done on MEGA during this period was divided between that done at Valparaiso University and that done at LAMPF. In addition, some contributions were made to a proposal to the LAMPF PAC to perform a precision measurement of the Michel ρ parameter, described below

  7. High sensitivity tests of the standard model for electroweak interactions

    International Nuclear Information System (INIS)

    1994-01-01

    The work done on this project focused on two LAMPF experiments. The MEGA experiment is a high-sensitivity search for the lepton family number violating decay μ → eγ to a sensitivity which, measured in terms of the branching ratio, BR = [μ → eγ]/[μ eν μ ν e ] ∼ 10 -13 , will be over two orders of magnitude better than previously reported values. The second is a precision measurement of the Michel ρ parameter from the positron energy spectrum of μ → eν μ ν e to test the predictions V-A theory of weak interactions. In this experiment the uncertainty in the measurement of the Michel ρ parameter is expected to be a factor of three lower than the present reported value. The detectors are operational, and data taking has begun

  8. High sensitivity tests of the standard model for electroweak interactions

    International Nuclear Information System (INIS)

    Koetke, D.D.; Manweiler, R.W.; Shirvel Stanislaus, T.D.

    1993-01-01

    The work done on this project was focused on two LAMPF experiments. The MEGA experiment, a high-sensitivity search for the lepton-family-number-violating decay μ → e γ to a sensitivity which, measured in terms of the branching ratio, BR = [μ → e γ]/[μ → ev μ v e ] ∼ 10 -13 , is over two orders of magnitude better than previously reported values. The second is a precision measurement of the Michel ρ parameter from the positron energy spectrum of μ → ev μ v e to test the V-A theory of weak interactions. The uncertainty in the measurement of the Michel ρ parameter is expected to be a factor of three lower than the present reported value

  9. Highly Sensitive Filter Paper Substrate for SERS Trace Explosives Detection

    Directory of Open Access Journals (Sweden)

    Pedro M. Fierro-Mercado

    2012-01-01

    Full Text Available We report on a novel and extremely low-cost surface-enhanced Raman spectroscopy (SERS substrate fabricated depositing gold nanoparticles on common lab filter paper using thermal inkjet technology. The paper-based substrate combines all advantages of other plasmonic structures fabricated by more elaborate techniques with the dynamic flexibility given by the inherent nature of the paper for an efficient sample collection, robustness, and stability. We describe the fabrication, characterization, and SERS activity of our substrate using 2,4,6-trinitrotoluene, 2,4-dinitrotoluene, and 1,3,5-trinitrobenzene as analytes. The paper-based SERS substrates presented a high sensitivity and excellent reproducibility for analytes employed, demonstrating a direct application in forensic science and homeland security.

  10. BH3105 type neutron dose equivalent meter of high sensitivity

    International Nuclear Information System (INIS)

    Ji Changsong; Zhang Enshan; Yang Jianfeng; Zhang Hong; Huang Jiling

    1995-10-01

    It is noted that to design a neutron dose meter of high sensitivity is almost impossible in the frame of traditional designing principle--'absorption net principle'. Based on a newly proposed principle of obtaining neutron dose equi-biological effect adjustment--' absorption stick principle', a brand-new neutron dose-equivalent meter with high neutron sensitivity BH3105 has been developed. Its sensitivity reaches 10 cps/(μSv·h -1 ), which is 18∼40 times higher than one of foreign products of the same kind and is 10 4 times higher than that of domestic FJ342 neutron rem-meter. BH3105 has a measurement range from 0.1μSv/h to 1 Sv/h which is 1 or 2 orders wider than that of the other's. It has the advanced properties of gamma-resistance, energy response, orientation, etc. (6 tabs., 5 figs.)

  11. High sensitive quench detection method using an integrated test wire

    International Nuclear Information System (INIS)

    Fevrier, A.; Tavergnier, J.P.; Nithart, H.; Kiblaire, M.; Duchateau, J.L.

    1981-01-01

    A high sensitive quench detection method which works even in the presence of an external perturbing magnetic field is reported. The quench signal is obtained from the difference in voltages at the superconducting winding terminals and at the terminals at a secondary winding strongly coupled to the primary. The secondary winding could consist of a ''zero-current strand'' of the superconducting cable not connected to one of the winding terminals or an integrated normal test wire inside the superconducting cable. Experimental results on quench detection obtained by this method are described. It is shown that the integrated test wire method leads to efficient and sensitive quench detection, especially in the presence of an external perturbing magnetic field

  12. A simple, tunable, and highly sensitive radio-frequency sensor.

    Science.gov (United States)

    Cui, Yan; Sun, Jiwei; He, Yuxi; Wang, Zheng; Wang, Pingshan

    2013-08-05

    We report a radio frequency (RF) sensor that exploits tunable attenuators and phase shifters to achieve high-sensitivity and broad band frequency tunability. Three frequency bands are combined to enable sensor operations from ∼20 MHz to ∼38 GHz. The effective quality factor ( Q eff ) of the sensor is as high as ∼3.8 × 10 6 with 200  μ l of water samples. We also demonstrate the measurement of 2-proponal-water-solution permittivity at 0.01 mole concentration level from ∼1 GHz to ∼10 GHz. Methanol-water solution and de-ionized water are used to calibrate the RF sensor for the quantitative measurements.

  13. Development of miniature γ dose rate monitor with high sensitivity

    International Nuclear Information System (INIS)

    Shi Huilu; Tuo Xianguo; Xi Dashun; Tang Rong; Mu Keliang; Yang Jianbo

    2009-01-01

    This paper introduces a miniature γ dose rate monitor with high sensitivity which design based on single chip microcomputer, it can continue monitoring γ dose rate and then choose wire or wireless communications to sent the monitoring data to host according to the actual conditions. It has two kinds of power supply system, AC power supply system and battery which can be chose by concrete circumstances. The design idea and implementation technology of hardware and software and the system structure of the monitor are detailed illustrated in this paper. The experimental results show that measurable range is 0.1 mR/h-200 mR/h, the sensitivity of γ is 90 cps/mR/h, dead time below 200 us, error of stability below ±10%. (authors)

  14. Wide bandwidth transimpedance amplifier for extremely high sensitivity continuous measurements.

    Science.gov (United States)

    Ferrari, Giorgio; Sampietro, Marco

    2007-09-01

    This article presents a wide bandwidth transimpedance amplifier based on the series of an integrator and a differentiator stage, having an additional feedback loop to discharge the standing current from the device under test (DUT) to ensure an unlimited measuring time opportunity when compared to switched discharge configurations while maintaining a large signal amplification over the full bandwidth. The amplifier shows a flat response from 0.6 Hz to 1.4 MHz, the capability to operate with leakage currents from the DUT as high as tens of nanoamperes, and rail-to-rail dynamic range for sinusoidal current signals independent of the DUT leakage current. Also available is a monitor output of the stationary current to track experimental slow drifts. The circuit is ideal for noise spectral and impedance measurements of nanodevices and biomolecules when in the presence of a physiological medium and in all cases where high sensitivity current measurements are requested such as in scanning probe microscopy systems.

  15. Development of High Sensitivity Nuclear Emulsion and Fine Grained Emulsion

    Science.gov (United States)

    Kawahara, H.; Asada, T.; Naka, T.; Naganawa, N.; Kuwabara, K.; Nakamura, M.

    2014-08-01

    Nuclear emulsion is a particle detector having high spacial resolution and angular resolution. It became useful for large statistics experiment thanks to the development of automatic scanning system. In 2010, a facility for emulsion production was introduced and R&D of nuclear emulsion began at Nagoya university. In this paper, we present results of development of the high sensitivity emulsion and fine grained emulsion for dark matter search experiment. Improvement of sensitivity is achieved by raising density of silver halide crystals and doping well-adjusted amount of chemicals. Production of fine grained emulsion was difficult because of unexpected crystal condensation. By mixing polyvinyl alcohol (PVA) to gelatin as a binder, we succeeded in making a stable fine grained emulsion.

  16. Development of High Sensitivity Nuclear Emulsion and Fine Grained Emulsion

    International Nuclear Information System (INIS)

    Kawahara, H.; Asada, T.; Naka, T.; Naganawa, N.; Kuwabara, K.; Nakamura, M.

    2014-01-01

    Nuclear emulsion is a particle detector having high spacial resolution and angular resolution. It became useful for large statistics experiment thanks to the development of automatic scanning system. In 2010, a facility for emulsion production was introduced and R and D of nuclear emulsion began at Nagoya university. In this paper, we present results of development of the high sensitivity emulsion and fine grained emulsion for dark matter search experiment. Improvement of sensitivity is achieved by raising density of silver halide crystals and doping well-adjusted amount of chemicals. Production of fine grained emulsion was difficult because of unexpected crystal condensation. By mixing polyvinyl alcohol (PVA) to gelatin as a binder, we succeeded in making a stable fine grained emulsion

  17. High-Sensitivity GaN Microchemical Sensors

    Science.gov (United States)

    Son, Kyung-ah; Yang, Baohua; Liao, Anna; Moon, Jeongsun; Prokopuk, Nicholas

    2009-01-01

    Systematic studies have been performed on the sensitivity of GaN HEMT (high electron mobility transistor) sensors using various gate electrode designs and operational parameters. The results here show that a higher sensitivity can be achieved with a larger W/L ratio (W = gate width, L = gate length) at a given D (D = source-drain distance), and multi-finger gate electrodes offer a higher sensitivity than a one-finger gate electrode. In terms of operating conditions, sensor sensitivity is strongly dependent on transconductance of the sensor. The highest sensitivity can be achieved at the gate voltage where the slope of the transconductance curve is the largest. This work provides critical information about how the gate electrode of a GaN HEMT, which has been identified as the most sensitive among GaN microsensors, needs to be designed, and what operation parameters should be used for high sensitivity detection.

  18. Effective dose calculation in CT using high sensitivity TLDs

    International Nuclear Information System (INIS)

    Brady, Z.; Johnston, P.N.

    2010-01-01

    Full text: To determine the effective dose for common paediatric CT examinations using thermoluminescence dosimetry (TLD) mea surements. High sensitivity TLD chips (LiF:Mg,Cu,P, TLD-IOOH, Thermo Fisher Scientific, Waltham, MA) were calibrated on a linac at an energy of 6 MY. A calibration was also performed on a superricial X-ray unit at a kilovoltage energy to validate the megavoltage cali bration for the purpose of measuring doses in the diagnostic energy range. The dose variation across large organs was assessed and a methodology for TLD placement in a 10 year old anthropomorphic phantom developed. Effective dose was calculated from the TLD measured absorbed doses for typical CT examinations after correcting for the TLD energy response and taking into account differences in the mass energy absorption coefficients for different tissues and organs. Results Using new tissue weighting factors recommended in ICRP Publication 103, the effective dose for a CT brain examination on a 10 year old was 1.6 millisieverts (mSv), 4.9 mSv for a CT chest exa ination and 4.7 mSv for a CT abdomen/pelvis examination. These values are lower for the CT brain examination, higher for the CT chest examination and approximately the same for the CT abdomen/ pelvis examination when compared with effective doses calculated using ICRP Publication 60 tissue weighting factors. Conclusions High sensitivity TLDs calibrated with a radiotherapy linac are useful for measuring dose in the diagnostic energy range and overcome limitations of output reproducibility and uniformity asso ciated with traditional TLD calibration on CT scanners or beam quality matched diagnostic X-ray units.

  19. Field test investigation of high sensitivity fiber optic seismic geophone

    Science.gov (United States)

    Wang, Meng; Min, Li; Zhang, Xiaolei; Zhang, Faxiang; Sun, Zhihui; Li, Shujuan; Wang, Chang; Zhao, Zhong; Hao, Guanghu

    2017-10-01

    Seismic reflection, whose measured signal is the artificial seismic waves ,is the most effective method and widely used in the geophysical prospecting. And this method can be used for exploration of oil, gas and coal. When a seismic wave travelling through the Earth encounters an interface between two materials with different acoustic impedances, some of the wave energy will reflect off the interface and some will refract through the interface. At its most basic, the seismic reflection technique consists of generating seismic waves and measuring the time taken for the waves to travel from the source, reflect off an interface and be detected by an array of geophones at the surface. Compared to traditional geophones such as electric, magnetic, mechanical and gas geophone, optical fiber geophones have many advantages. Optical fiber geophones can achieve sensing and signal transmission simultaneously. With the development of fiber grating sensor technology, fiber bragg grating (FBG) is being applied in seismic exploration and draws more and more attention to its advantage of anti-electromagnetic interference, high sensitivity and insensitivity to meteorological conditions. In this paper, we designed a high sensitivity geophone and tested its sensitivity, based on the theory of FBG sensing. The frequency response range is from 10 Hz to 100 Hz and the acceleration of the fiber optic seismic geophone is over 1000pm/g. sixteen-element fiber optic seismic geophone array system is presented and the field test is performed in Shengli oilfield of China. The field test shows that: (1) the fiber optic seismic geophone has a higher sensitivity than the traditional geophone between 1-100 Hz;(2) The low frequency reflection wave continuity of fiber Bragg grating geophone is better.

  20. A CMOS In-Pixel CTIA High Sensitivity Fluorescence Imager.

    Science.gov (United States)

    Murari, Kartikeya; Etienne-Cummings, Ralph; Thakor, Nitish; Cauwenberghs, Gert

    2011-10-01

    Traditionally, charge coupled device (CCD) based image sensors have held sway over the field of biomedical imaging. Complementary metal oxide semiconductor (CMOS) based imagers so far lack sensitivity leading to poor low-light imaging. Certain applications including our work on animal-mountable systems for imaging in awake and unrestrained rodents require the high sensitivity and image quality of CCDs and the low power consumption, flexibility and compactness of CMOS imagers. We present a 132×124 high sensitivity imager array with a 20.1 μm pixel pitch fabricated in a standard 0.5 μ CMOS process. The chip incorporates n-well/p-sub photodiodes, capacitive transimpedance amplifier (CTIA) based in-pixel amplification, pixel scanners and delta differencing circuits. The 5-transistor all-nMOS pixel interfaces with peripheral pMOS transistors for column-parallel CTIA. At 70 fps, the array has a minimum detectable signal of 4 nW/cm(2) at a wavelength of 450 nm while consuming 718 μA from a 3.3 V supply. Peak signal to noise ratio (SNR) was 44 dB at an incident intensity of 1 μW/cm(2). Implementing 4×4 binning allowed the frame rate to be increased to 675 fps. Alternately, sensitivity could be increased to detect about 0.8 nW/cm(2) while maintaining 70 fps. The chip was used to image single cell fluorescence at 28 fps with an average SNR of 32 dB. For comparison, a cooled CCD camera imaged the same cell at 20 fps with an average SNR of 33.2 dB under the same illumination while consuming over a watt.

  1. Atomic population redistribution in a dense Ga vapour proceeding via energy pooling ionization induced by resonant laser-assisted collisions

    International Nuclear Information System (INIS)

    Barsanti, S; Bicchi, P

    2002-01-01

    In this paper we report on the atomic population redistribution originating from the ionization that takes place in a dense Ga vapour kept in quartz cells and resonantly excited by laser radiation, in the collisions between two excited atoms. This ionization process is known as energy-pooling ionization (EPI). The electron/ion recombination that takes place in the low density plasma produced gives rise to population in the atomic Rydberg levels and from the latter via cascade transitions to lower lying ones. We have monitored the fluorescences relative to the radiative emissions from such levels, namely those corresponding to the nP → 5S 1/2 series, with 9 ≤ n ≤ 26, and the 4D → 4P 1/2,3/2 transitions. Their characteristics testify to their origin as being due to the EPI process. Further confirmation is obtained by performing a time-resolved analysis of such fluorescences, whose appearance and time evolution is strongly influenced by the dynamics of the process. The effect of the introduction of a few Torr of buffer gas inside the quartz cell, resulting in the quenching of all the fluorescences for n ≥ 12, is also discussed

  2. High sensitivity 1H-NMR spectroscopy of homeopathic remedies made in water

    Science.gov (United States)

    Anick, David J

    2004-01-01

    Background The efficacy of homeopathy is controversial. Homeopathic remedies are made via iterated shaking and dilution, in ethanol or in water, from a starting substance. Remedies of potency 12 C or higher are ultra-dilute (UD), i.e. contain zero molecules of the starting material. Various hypotheses have been advanced to explain how a UD remedy might be different from unprepared solvent. One such hypothesis posits that a remedy contains stable clusters, i.e. localized regions where one or more hydrogen bonds remain fixed on a long time scale. High sensitivity proton nuclear magnetic resonance spectroscopy has not previously been used to look for evidence of differences between UD remedies and controls. Methods Homeopathic remedies made in water were studied via high sensitivity proton nuclear magnetic resonance spectroscopy. A total of 57 remedy samples representing six starting materials and spanning a variety of potencies from 6 C to 10 M were tested along with 46 controls. Results By presaturating on the water peak, signals could be reliably detected that represented H-containing species at concentrations as low as 5 μM. There were 35 positions where a discrete signal was seen in one or more of the 103 spectra, which should theoretically have been absent from the spectrum of pure water. Of these 35, fifteen were identified as machine-generated artifacts, eight were identified as trace levels of organic contaminants, and twelve were unexplained. Of the unexplained signals, six were seen in just one spectrum each. None of the artifacts or unexplained signals occurred more frequently in remedies than in controls, using a p < .05 cutoff. Some commercially prepared samples were found to contain traces of one or more of these small organic molecules: ethanol, acetate, formate, methanol, and acetone. Conclusion No discrete signals suggesting a difference between remedies and controls were seen, via high sensitivity 1H-NMR spectroscopy. The results failed to support

  3. Synchronisation of self-oscillations in a solid-state ring laser with pump modulation in the region of parametric resonance between self-modulation and relaxation oscillations

    International Nuclear Information System (INIS)

    Dudetskiy, V Yu; Lariontsev, E G; Chekina, S N

    2014-01-01

    The synchronisation of the self-modulation oscillation frequency in a Nd : YAG ring laser by an external periodic signal modulating the pump power in the region of parametric resonance between self-modulation and relaxation oscillations is studied theoretically and experimentally. The characteristic features of synchronisation processes in lasers operating in the self-modulation regime of the first kind and in the regime with a doubled self-modulation period are considered. Two bistable branches of synchronisation of self-modulation oscillations are found by numerical calculation. The experimental data agree well with the numerical simulation results for one of these branches, but the other branch of bistable self-modulation oscillations was not observed experimentally. (control of laser radiation parameters)

  4. Spectroscopic studies on technetium and silicon. A solid-state laser system for the resonance-ionization spectroscopy; Spektroskopische Untersuchungen an Technetium und Silizium. Ein Festkoerperlasersystem fuer die Resonanzionisationsspektroskopie

    Energy Technology Data Exchange (ETDEWEB)

    Mattolat, Christoph

    2010-11-15

    This doctoral thesis describes advancement and refinement of the titanium:sapphire laser system of the working group LARISSA, Institut fuer Physik, Johannes Gutenberg- Universitaet Mainz and its application to resonance ionization spectroscopy. Activities on the laser systems comprised three major tasks: The output power of the conventional titanium:sapphire lasers could be increased by a factor of two in order to match the needs at resonance ionization laser ion source at ISOL facilities. Additionally, the laser system was complemented by a titanium:sapphire laser in Littrow geometry, which ensures a mode-hop free tuning range from 700 nm to 950 nm, and by an injection seeded titanium:sapphire laser with a spectral width of 20 MHz (in respect to a spectral width of 3 GHz for the conventional lasers). The performance of the new laser system was tested in spectroscopic investigations of highly excited atomic levels of gold and technetium. From the measured level positions the ionization potential of gold could be verified by using the Rydberg-Ritz formula, while the ionization potential of technetium could be determined precisely for the first time. Using the seeded titanium: sapphire laser Doppler-free two-photon spectroscopy inside a hot ionizer cavity was demonstrated. A width of the recorded resonances of 90 MHz was achieved and the hyperfine structure and isotope shift of stable silicon isotopes was well resolved with this method. (orig.)

  5. Storing quantum information in spins and high-sensitivity ESR.

    Science.gov (United States)

    Morton, John J L; Bertet, Patrice

    2018-02-01

    Quantum information, encoded within the states of quantum systems, represents a novel and rich form of information which has inspired new types of computers and communications systems. Many diverse electron spin systems have been studied with a view to storing quantum information, including molecular radicals, point defects and impurities in inorganic systems, and quantum dots in semiconductor devices. In these systems, spin coherence times can exceed seconds, single spins can be addressed through electrical and optical methods, and new spin systems with advantageous properties continue to be identified. Spin ensembles strongly coupled to microwave resonators can, in principle, be used to store the coherent states of single microwave photons, enabling so-called microwave quantum memories. We discuss key requirements in realising such memories, including considerations for superconducting resonators whose frequency can be tuned onto resonance with the spins. Finally, progress towards microwave quantum memories and other developments in the field of superconducting quantum devices are being used to push the limits of sensitivity of inductively-detected electron spin resonance. The state-of-the-art currently stands at around 65 spins per Hz, with prospects to scale down to even fewer spins. Copyright © 2017. Published by Elsevier Inc.

  6. Storing quantum information in spins and high-sensitivity ESR

    Science.gov (United States)

    Morton, John J. L.; Bertet, Patrice

    2018-02-01

    Quantum information, encoded within the states of quantum systems, represents a novel and rich form of information which has inspired new types of computers and communications systems. Many diverse electron spin systems have been studied with a view to storing quantum information, including molecular radicals, point defects and impurities in inorganic systems, and quantum dots in semiconductor devices. In these systems, spin coherence times can exceed seconds, single spins can be addressed through electrical and optical methods, and new spin systems with advantageous properties continue to be identified. Spin ensembles strongly coupled to microwave resonators can, in principle, be used to store the coherent states of single microwave photons, enabling so-called microwave quantum memories. We discuss key requirements in realising such memories, including considerations for superconducting resonators whose frequency can be tuned onto resonance with the spins. Finally, progress towards microwave quantum memories and other developments in the field of superconducting quantum devices are being used to push the limits of sensitivity of inductively-detected electron spin resonance. The state-of-the-art currently stands at around 65 spins per √{ Hz } , with prospects to scale down to even fewer spins.

  7. X-ray comb generation from nuclear-resonance-stabilized x-ray free-electron laser oscillator for fundamental physics and precision metrology

    Directory of Open Access Journals (Sweden)

    B. W. Adams

    2015-03-01

    Full Text Available An x-ray free-electron laser oscillator (XFELO is a next-generation x-ray source, similar to free-electron laser oscillators at VUV and longer wavelengths but using crystals as high-reflectivity x-ray mirrors. Each output pulse from an XFELO is fully coherent with high spectral purity. The temporal coherence length can further be increased drastically, from picoseconds to microseconds or even longer, by phase-locking successive XFELO output pulses, using the narrow nuclear resonance lines of nuclei such as ^{57}Fe as a reference. We show that the phase fluctuation due to the seismic activities is controllable and that due to spontaneous emission is small. The fluctuation of electron-bunch spacing contributes mainly to the envelope fluctuation but not to the phase fluctuation. By counting the number of standing-wave maxima formed by the output of the nuclear-resonance-stabilized (NRS XFELO over an optically known length, the wavelength of the nuclear resonance can be accurately measured, possibly leading to a new length or frequency standard at x-ray wavelengths. A NRS-XFELO will be an ideal source for experimental x-ray quantum optics as well as other fundamental physics. The technique can be refined for other, narrower resonances such as ^{181}Ta or ^{45}Sc.

  8. Domain Engineered Magnetoelectric Thin Films for High Sensitivity Resonant Magnetic Field Sensors

    Science.gov (United States)

    2012-02-28

    increas small at low uency shift ur hypothes former: Sin (output), w tion. Materia ansducer. Th e transform voltage gai rmer. Furth ansformer p ded...90 min, r 0 Oe to 300 ith increasin ity (GH-G0/G tic field. Th dels. The d agnetic fiel ion of actua rent materia se with high nce and new r. This

  9. Domain Engineered Magnetoelectric Thin Films for High Sensitivity Resonant Magnetic Field Sensors

    Science.gov (United States)

    2011-12-01

    band gap of highly textured PZT thin films. The deposition process variables were - argon and oxygen flows, chamber pressure, RF power (DC Bias...needed another parameter to equate with the number of unknowns in the resultant model equations. From Figure 24, electronic polarizability affects the... Polarizability and Optical dielectric response of a thin.film , ., ,__~--~---\\- 000 01’ "󈧶 Ots Tncnt.re"’°l Effective Polarizability = Reddy

  10. CRDS with a VECSEL for broad-band high sensitivity spectroscopy in the 2.3 μm window

    Energy Technology Data Exchange (ETDEWEB)

    Čermák, P., E-mail: cermak@fmph.uniba.sk [University Grenoble Alpes, LIPhy, F-38000 Grenoble (France); CNRS, LIPhy, UMR 5588, F-38000 Grenoble (France); Department of Experimental Physics, Faculty of Mathematics, Physics and Informatics, Comenius University, Mlynská Dolina, 842 48 Bratislava (Slovakia); Chomet, B. [IES, CNRS, UMR5214, University Montpellier, F-34000 Montpellier (France); Innoptics, Institut d’Optique d’Aquitaine Rue François Mitterrand, 33400 Talence (France); Ferrieres, L.; Denet, S.; Lecocq, V. [Innoptics, Institut d’Optique d’Aquitaine Rue François Mitterrand, 33400 Talence (France); Vasilchenko, S. [University Grenoble Alpes, LIPhy, F-38000 Grenoble (France); CNRS, LIPhy, UMR 5588, F-38000 Grenoble (France); Laboratory of Molecular Spectroscopy, V.E. Zuev Institute of Atmospheric Optics, SB Russian Academy of Science, 1 Academician Zuev Square, 634021 Tomsk (Russian Federation); Mondelain, D.; Kassi, S.; Campargue, A. [University Grenoble Alpes, LIPhy, F-38000 Grenoble (France); CNRS, LIPhy, UMR 5588, F-38000 Grenoble (France); Myara, M.; Cerutti, L.; Garnache, A. [IES, CNRS, UMR5214, University Montpellier, F-34000 Montpellier (France)

    2016-08-15

    The integration of an industry ready packaged Sb-based Vertical-External-Cavity Surface-Emitting-Laser (VECSEL) into a Cavity Ring Down Spectrometer (CRDS) is presented. The instrument operates in the important 2.3 μm atmospheric transparency window and provides a high sensitivity (minimum detectable absorption of 9 × 10{sup −11} cm{sup −1}) over a wide spectra range. The VECSEL performances combine a large continuous tunability over 120 cm{sup −1} around 4300 cm{sup −1} together with a powerful (∼5 mW) TEM{sub 00} diffraction limited beam and linewidth at MHz level (for 1 ms of integration time). The achieved performances are illustrated by high sensitivity recordings of the very weak absorption spectrum of water vapor in the region. The developed method gives potential access to the 2-2.7 μm range for CRDS.

  11. CRDS with a VECSEL for broad-band high sensitivity spectroscopy in the 2.3 μm window.

    Science.gov (United States)

    Čermák, P; Chomet, B; Ferrieres, L; Vasilchenko, S; Mondelain, D; Kassi, S; Campargue, A; Denet, S; Lecocq, V; Myara, M; Cerutti, L; Garnache, A

    2016-08-01

    The integration of an industry ready packaged Sb-based Vertical-External-Cavity Surface-Emitting-Laser (VECSEL) into a Cavity Ring Down Spectrometer (CRDS) is presented. The instrument operates in the important 2.3 μm atmospheric transparency window and provides a high sensitivity (minimum detectable absorption of 9 × 10(-11) cm(-1)) over a wide spectra range. The VECSEL performances combine a large continuous tunability over 120 cm(-1) around 4300 cm(-1) together with a powerful (∼5 mW) TEM00 diffraction limited beam and linewidth at MHz level (for 1 ms of integration time). The achieved performances are illustrated by high sensitivity recordings of the very weak absorption spectrum of water vapor in the region. The developed method gives potential access to the 2-2.7 μm range for CRDS.

  12. Generation of Raman lasers from nitrogen molecular ions driven by ultraintense laser fields

    Science.gov (United States)

    Yao, Jinping; Chu, Wei; Liu, Zhaoxiang; Xu, Bo; Chen, Jinming; Cheng, Ya

    2018-03-01

    Atmospheric lasing has aroused much interest in the past few years. The ‘air–laser’ opens promising potential for remote chemical sensing of trace gases with high sensitivity and specificity. At present, several approaches have been successfully implemented for generating highly coherent laser beams in atmospheric condition, including both amplified-spontaneous emission, and narrow-bandwidth stimulated emission in the forward direction in the presence of self-generated or externally injected seed pulses. Here, we report on generation of multiple-wavelength Raman lasers from nitrogen molecular ions ({{{N}}}2+), driven by intense mid-infrared laser fields. Intuitively, the approach appears problematic for the small nonlinear susceptibility of {{{N}}}2+ ions, whereas the efficiency of Raman laser can be significantly promoted in near-resonant condition. More surprisingly, a Raman laser consisting of a supercontinuum spanning from ∼310 to ∼392 nm has been observed resulting from a series near-resonant nonlinear processes including four-wave mixing, stimulated Raman scattering and cross phase modulation. To date, extreme nonlinear optics in molecular ions remains largely unexplored, which provides an alternative means for air–laser-based remote sensing applications.

  13. A laser gyro with a four-mirror square resonator: formulas for simulating the dynamics of the synchronisation zone parameters of the frequencies of counterpropagating waves during the device operation in the self-heating regime

    International Nuclear Information System (INIS)

    Bondarenko, E A

    2014-01-01

    For a laser gyro with a four-mirror square resonator we have developed a mathematical model, which allows one to simulate the temporal behaviour of the synchronisation zone parameters of the frequencies of counterpropagating waves in a situation when the device operates in the self-heating regime and is switched-on at different initial temperatures. (laser gyroscopes)

  14. Polypyrrole–gold nanoparticle composites for highly sensitive DNA detection

    International Nuclear Information System (INIS)

    Spain, Elaine; Keyes, Tia E.; Forster, Robert J.

    2013-01-01

    DNA capture surfaces represent a powerful approach to developing highly sensitive sensors for identifying the cause of infection. Electrochemically deposited polypyrrole, PPy, films have been functionalized with electrodeposited gold nanoparticles to give a nanocomposite material, PPy–AuNP. Thiolated capture strand DNA, that is complementary to the sequence from the pathogen Staphylococcus aureus that causes mammary gland inflammation, was then immobilized onto the gold nanoparticles and any of the underlying gold electrode that is exposed. A probe strand, labelled with horse radish peroxidase, HRP, was then hybridized to the target. The concentration of the target was determined by measuring the current generated by reducing benzoquinone produced by the HRP label. Semi-log plots of the pathogen DNA concentration vs. faradaic current are linear from 150 pM to 1 μM and pM concentrations can be detected without the need for molecular, e.g., PCR or NASBA, amplification. The nanocomposite also exhibits excellent selectivity and single base mismatches in a 30 mer sequence can be detected

  15. Operationalization of the Russian Version of Highly Sensitive Person Scale

    Directory of Open Access Journals (Sweden)

    Регина Вячеславовна Ершова

    2018-12-01

    Full Text Available The aim of the present study was to operationalize a Russian version of the Highly Sensitive Person Scale (HSPS. The empirical data were collected in two ways: active, through oral advertising and inviting those who wish to take part in the study (snowball technique and passive (placement of ads about taking part in a research in social networks VKontakte and Facebook. As a result, 350 university students (117 men, 233 women, an average age of 18,2 (± 1,7 applied to a research laboratory and filled out the HSPS questionnaire, and another 510 respondents (380 women, 130 men, average age 22,6 ( ± 7,9 filled the HSPS online. The results of the study did not confirm the one-dimensional model of the construct, proposed by Aron & Aron (1997, as well as the most commonly used in the English-language studies three-factor solution. The hierarchical claster and confirmatory analyses used in the operationalization procedure allowed us to conclude that the variance of the Russian version of HSPS is best described in the framework of a two-factor model including the two separate subscales: Ease of Excitation (EOE, Low threshold of sensitivity (LTS. Sensory Processing Sensitivity may be defined as an increased susceptibility to external and internal stimuli, realized through negative emotional responses and deep susceptibility (distress to excessive stimulation.

  16. Luminescent Lanthanide Reporters for High-Sensitivity Novel Bioassays

    Energy Technology Data Exchange (ETDEWEB)

    Anstey, Mitchell R. [Sandia National Lab. (SNL-CA), Livermore, CA (United States); Fruetel, Julia A. [Sandia National Lab. (SNL-CA), Livermore, CA (United States); Foster, Michael E. [Sandia National Lab. (SNL-CA), Livermore, CA (United States); Hayden, Carl C. [Sandia National Lab. (SNL-CA), Livermore, CA (United States); Buckley, Heather L. [Sandia National Lab. (SNL-CA), Livermore, CA (United States); Arnold, John [Sandia National Lab. (SNL-CA), Livermore, CA (United States)

    2013-09-01

    Biological imaging and assay technologies rely on fluorescent organic dyes as reporters for a number of interesting targets and processes. However, limitations of organic dyes such as small Stokes shifts, spectral overlap of emission signals with native biological fluorescence background, and photobleaching have all inhibited the development of highly sensitive assays. To overcome the limitations of organic dyes for bioassays, we propose to develop lanthanide-based luminescent dyes and demonstrate them for molecular reporting applications. This relatively new family of dyes was selected for their attractive spectral and chemical properties. Luminescence is imparted by the lanthanide atom and allows for relatively simple chemical structures that can be tailored to the application. The photophysical properties offer unique features such as narrow and non-overlapping emission bands, long luminescent lifetimes, and long wavelength emission, which enable significant sensitivity improvements over organic dyes through spectral and temporal gating of the luminescent signal.Growth in this field has been hindered due to the necessary advanced synthetic chemistry techniques and access to experts in biological assay development. Our strategy for the development of a new lanthanide-based fluorescent reporter system is based on chelation of the lanthanide metal center using absorbing chromophores. Our first strategy involves "Click" chemistry to develop 3-fold symmetric chelators and the other involves use of a new class of tetrapyrrole ligands called corroles. This two-pronged approach is geared towards the optimization of chromophores to enhance light output.

  17. Highly sensitive MoS2 photodetectors with graphene contacts

    Science.gov (United States)

    Han, Peize; St. Marie, Luke; Wang, Qing X.; Quirk, Nicholas; El Fatimy, Abdel; Ishigami, Masahiro; Barbara, Paola

    2018-05-01

    Two-dimensional materials such as graphene and transition metal dichalcogenides (TMDs) are ideal candidates to create ultra-thin electronics suitable for flexible substrates. Although optoelectronic devices based on TMDs have demonstrated remarkable performance, scalability is still a significant issue. Most devices are created using techniques that are not suitable for mass production, such as mechanical exfoliation of monolayer flakes and patterning by electron-beam lithography. Here we show that large-area MoS2 grown by chemical vapor deposition and patterned by photolithography yields highly sensitive photodetectors, with record shot-noise-limited detectivities of 8.7 × 1014 Jones in ambient condition and even higher when sealed with a protective layer. These detectivity values are higher than the highest values reported for photodetectors based on exfoliated MoS2. We study MoS2 devices with gold electrodes and graphene electrodes. The devices with graphene electrodes have a tunable band alignment and are especially attractive for scalable ultra-thin flexible optoelectronics.

  18. High-sensitivity bend angle measurements using optical fiber gratings.

    Science.gov (United States)

    Rauf, Abdul; Zhao, Jianlin; Jiang, Biqiang

    2013-07-20

    We present a high-sensitivity and more flexible bend measurement method, which is based on the coupling of core mode to the cladding modes at the bending region in concatenation with optical fiber grating serving as band reflector. The characteristics of a bend sensing arm composed of bending region and optical fiber grating is examined for different configurations including single fiber Bragg grating (FBG), chirped FBG (CFBG), and double FBGs. The bend loss curves for coated, stripped, and etched sections of fiber in the bending region with FBG, CFBG, and double FBG are obtained experimentally. The effect of separation between bending region and optical fiber grating on loss is measured. The loss responses for single FBG and CFBG configurations are compared to discover the effectiveness for practical applications. It is demonstrated that the sensitivity of the double FBG scheme is twice that of the single FBG and CFBG configurations, and hence acts as sensitivity multiplier. The bend loss response for different fiber diameters obtained through etching in 40% hydrofluoric acid, is measured in double FBG scheme that resulted in a significant increase in the sensitivity, and reduction of dead-zone.

  19. Highly sensitive BTX detection using surface functionalized QCM sensor

    Energy Technology Data Exchange (ETDEWEB)

    Bozkurt, Asuman Aşıkoğlu; Özdemir, Okan; Altındal, Ahmet, E-mail: altindal@yildiz.edu.tr [Department of Physics, Yildiz Technical University, Davutpasa, 34210 Istanbul (Turkey)

    2016-03-25

    A novel organic compound was designed and successfully synthesized for the fabrication of QCM based sensors to detect the low concentrations of BTX gases in indoor air. The effect of the long-range electron orbital delocalization on the BTX vapour sensing properties of azo-bridged Pcs based chemiresistor-type sensors have also been investigated in this work. The sensing behaviour of the film for the online detection of volatile organic solvent vapors was investigated by utilizing an AT-cut quartz crystal resonator. It was observed that the adsorption of the target molecules on the coating surface cause a reversible negative frequency shift of the resonator. Thus, a variety of solvent vapors can be detected by using the phthalocyanine film as sensitive coating, with sensitivity in the ppm range and response times in the order of several seconds depending on the molecular structure of the organic solvent.

  20. High-Q Fabry–Pérot Micro-Cavities for High-Sensitivity Volume Refractometry

    Directory of Open Access Journals (Sweden)

    Noha Gaber

    2018-01-01

    Full Text Available This work reports a novel structure for a Fabry–Pérot micro cavity that combines the highest reported quality factor for an on-chip Fabry–Pérot resonator that exceeds 9800, and a very high sensitivity for an on-chip volume refractometer based on a Fabry–Pérot cavity that is about 1000 nm/refractive index unit (RIU. The structure consists of two cylindrical Bragg micromirrors that achieve confinement of the Gaussian beam in the plan parallel to the chip substrate, while for the perpendicular plan, external fiber rod lenses (FRLs are placed in the optical path of the input and the output of the cavity. This novel structure overcomes number of the drawbacks presented in previous designs. The analyte is passed between the mirrors, enabling its detection from the resonance peak wavelengths of the transmission spectra. Mixtures of ethanol and deionized (DI-water with different ratios are used as analytes with different refractive indices to exploit the device as a micro-opto-fluidic refractometer. The design criteria are detailed and the modeling is based on Gaussian-optics equations, which depicts a scenario closer to reality than the usually used ray-optics modeling.

  1. Tumor-specific antivascular effect of TZT-1027 (Soblidotin) elucidated by magnetic resonance imaging and confocal laser scanning microscopy

    International Nuclear Information System (INIS)

    Natsume, Tsugitaka; Watanabe, Junichi; Kobayashi, Motohiro; Ogawa, Kenji; Yasumura, Kazuhiko

    2007-01-01

    TZT-1027 (soblidotin), an antimicrotubule agent, has previously been evaluated in terms of its antivascular effects. In this study, Evans blue perfusion, magnetic resonance imaging (MRI), and confocal laser scanning microscopy (CLSM) were utilized to further elucidate the antivascular effect of TZT-1027 in female nude mice and rats bearing human breast tumor MX-1, as well as in female Sprague-Dawley rats that developed breast tumors induced by dimethylbenz(a)anthracene (DMBA). Therapeutic doses of TZT-1027 caused nearly complete regression of implanted MX-1 tumors in nude mice and rats as well as DMBA-induced tumors in rats. The perfusion in MX-1 tumor implanted in nude mice was drastically reduced within 30 min after TZT-1027 administration and was completely inhibited after 6 h or more, although not reduced in normal tissue of kidney. The study using MRI demonstrated that rich blood flow within tumors was remarkably reduced 1-3 h after TZT-1027 administration both in nude rats bearing MX-1 tumors and in rats with DMBA-induced tumors. Furthermore, the study with CLSM in nude mice bearing MX-1 tumors revealed a disruption of tumor microvessels at 1 h and a destruction of tumor microvessel network at 3 h after TZT-1027 administration. In contrast, these types of vascular disorders were not observed in heart and kidney. These results suggest that TZT-1027 specifically damages tumor vasculatures, leading to extensive tumor necrosis within tolerable dose range, and confirms earlier observations that TZT-1027 exerts a considerable antivascular effect in addition to an excellent cytotoxic effect. (author)

  2. Hair sparing does not compromise real-time magnetic resonance imaging guided stereotactic laser fiber placement for temporal lobe epilepsy.

    Science.gov (United States)

    Singh, Shikha; Kumar, Kevin K; Rabon, Matthew J; Dolce, Dana; Halpern, Casey H

    2018-06-01

    Pre-operative scalp shaving is conventionally thought to simplify postoperative cranial wound care, lower the rate of wound infections, and ease optimal incision localization. Over the past few decades, some neurosurgeons have refrained from scalp shaving in order to improve patient satisfaction with brain surgery. However, this hair-sparing approach has not yet been explored in the growing field of magnetic resonance-guided laser interstitial thermal therapy (MRgLITT). This study investigated the initial impact of a no-shave technique on post-operative wound infection rate as well as on entry and target accuracy in MRgLITT for mesial temporal epilepsy. Eighteen patients selected by the Stanford Comprehensive Epilepsy Program between November 2015 and August 2017 were included in the study. All patients underwent functional selective amygdalohippocampotomies using MRgLITT entirely within a diagnostic MRI suite. No hair was removed and no additional precautions were taken for hair or scalp care. Otherwise, routine protocols for surgical preparations and wound closure were followed. The study was performed under approval from Stanford University's Internal Review Board (IRB-37830). No post-operative wound infections or erosions occurred for any patient. The mean entry point error was 2.87 ± 1.3 mm and the mean target error was 1.0 ± 0.9 mm. There have been no other complications associated with this hair-sparing approach. The study's results suggest that hair sparing in MRgLITT surgery for temporal epilepsy does not increase the risk of wound complications or compromise accuracy. This preferred cosmetic approach may thus appeal to epilepsy patients considering such interventions. Copyright © 2018 Elsevier Ltd. All rights reserved.

  3. Lasers '90: Proceedings of the 13th International Conference on Lasers and Applications, San Diego, CA, Dec. 10-14, 1990

    International Nuclear Information System (INIS)

    Harris, D.G.; Herbelin, J.

    1991-01-01

    The general topics considered are: x-ray lasers; FELs; solid state lasers; techniques and phenomena of ultrafast lasers; optical filters and free space laser communications; discharge lasers; tunable lasers; applications of lasers in medicine and surgery; lasers in materials processing; high power lasers; dynamics gratings, wave mixing, and holography; up-conversion lasers; lidar and laser radar; laser resonators; excimer lasers; laser propagation; nonlinear and quantum optics; blue-green technology; imaging; laser spectroscopy; chemical lasers; dye lasers; and lasers in chemistry

  4. High sensitivity fiber optic angular displacement sensor and its application for detection of ultrasound.

    Science.gov (United States)

    Sakamoto, João Marcos Salvi; Kitano, Cláudio; Pacheco, Gefeson Mendes; Tittmann, Bernhard Rainer

    2012-07-10

    In this paper, we report on the development of an intensity-modulated fiber-optic sensor for angular displacement measurement. This sensor was designed to present high sensitivity, linear response, and wide bandwidth and, furthermore, to be simple and low cost. The sensor comprises two optical fibers, a positive lens, a reflective surface, an optical source, and a photodetector. A mathematical model was developed to determine and simulate the static characteristic curve of the sensor and to compare different sensor configurations regarding the core radii of the optical fibers. The simulation results showed that the sensor configurations tested are highly sensitive to small angle variation (in the range of microradians) with nonlinearity less than or equal to 1%. The normalized sensitivity ranges from (0.25×V(max)) to (2.40×V(max)) mV/μrad (where V(max) is the peak voltage of the static characteristic curve), and the linear range is from 194 to 1840 μrad. The unnormalized sensitivity for a reflective surface with reflectivity of 100% was measured as 7.7 mV/μrad. The simulations were compared with experimental results to validate the mathematical model and to define the most suitable configuration for ultrasonic detection. The sensor was tested on the characterization of a piezoelectric transducer and as part of a laser ultrasonics setup. The velocities of the longitudinal, shear, and surface waves were measured on aluminum samples as 6.43, 3.17, and 2.96 mm/μs, respectively, with an error smaller than 1.3%. The sensor, an alternative to piezoelectric or interferometric detectors, proved to be suitable for detection of ultrasonic waves and to perform time-of-flight measurements and nondestructive inspection.

  5. High Sensitivity Refractometer Based on TiO2-Coated Adiabatic Tapered Optical Fiber via ALD Technology

    Science.gov (United States)

    Zhu, Shan; Pang, Fufei; Huang, Sujuan; Zou, Fang; Guo, Qiang; Wen, Jianxiang; Wang, Tingyun

    2016-01-01

    Atomic layer deposition (ALD) technology is introduced to fabricate a high sensitivity refractometer based on an adiabatic tapered optical fiber. Different thicknesses of titanium dioxide (TiO2) nanofilm were coated around the tapered fiber precisely and uniformly under different deposition cycles. Attributed to the higher refractive index of the TiO2 nanofilm compared to that of silica, an asymmetric Fabry–Perot (F-P) resonator could be constructed along the fiber taper. The central wavelength of the F-P resonator could be controlled by adjusting the thickness of the TiO2 nanofilm. Such a F-P resonator is sensitive to changes in the surrounding refractive index (SRI), which is utilized to realize a high sensitivity refractometer. The refractometer developed by depositing 50.9-nm-thickness TiO2 on the tapered fiber shows SRI sensitivity as high as 7096 nm/RIU in the SRI range of 1.3373–1.3500. Due to TiO2’s advantages of high refractive index, lack of toxicity, and good biocompatibility, this refractometer is expected to have wide applications in the biochemical sensing field. PMID:27537885

  6. High-Sensitivity Measurement of Density by Magnetic Levitation.

    Science.gov (United States)

    Nemiroski, Alex; Kumar, A A; Soh, Siowling; Harburg, Daniel V; Yu, Hai-Dong; Whitesides, George M

    2016-03-01

    This paper presents methods that use Magnetic Levitation (MagLev) to measure very small differences in density of solid diamagnetic objects suspended in a paramagnetic medium. Previous work in this field has shown that, while it is a convenient method, standard MagLev (i.e., where the direction of magnetization and gravitational force are parallel) cannot resolve differences in density mm) because (i) objects close in density prevent each other from reaching an equilibrium height due to hard contact and excluded volume, and (ii) using weaker magnets or reducing the magnetic susceptibility of the medium destabilizes the magnetic trap. The present work investigates the use of weak magnetic gradients parallel to the faces of the magnets as a means of increasing the sensitivity of MagLev without destabilization. Configuring the MagLev device in a rotated state (i.e., where the direction of magnetization and gravitational force are perpendicular) relative to the standard configuration enables simple measurements along the axes with the highest sensitivity to changes in density. Manipulating the distance of separation between the magnets or the lengths of the magnets (along the axis of measurement) enables the sensitivity to be tuned. These modifications enable an improvement in the resolution up to 100-fold over the standard configuration, and measurements with resolution down to 10(-6) g/cm(3). Three examples of characterizing the small differences in density among samples of materials having ostensibly indistinguishable densities-Nylon spheres, PMMA spheres, and drug spheres-demonstrate the applicability of rotated Maglev to measuring the density of small (0.1-1 mm) objects with high sensitivity. This capability will be useful in materials science, separations, and quality control of manufactured objects.

  7. High-sensitivity Cardiac Troponin Elevation after Electroconvulsive Therapy (ECT)

    Science.gov (United States)

    Duma, Andreas; Pal, Swatilika; Johnston, Joshua; Helwani, Mohammad A.; Bhat, Adithya; Gill, Bali; Rosenkvist, Jessica; Cartmill, Christopher; Brown, Frank; Miller, J. Philip; Scott, Mitchell G; Sanchez-Conde, Francisco; Jarvis, Michael; Farber, Nuri B.; Zorumski, Charles F.; Conway, Charles; Nagele, Peter

    2017-01-01

    Background While electroconvulsive therapy (ECT) is widely regarded as a life-saving and safe procedure, evidence regarding its effects on myocardial cell injury are sparse. The objective of this investigation was to determine incidence and magnitude of new cardiac troponin elevation after ECT using a novel high-sensitivity cardiac troponin I (hscTnI) assay. Methods This was a prospective cohort study in adult patients undergoing ECT in a single academic center (up to three ECT treatments per patient). The primary outcome was new hscTnI elevation after ECT, defined as an increase of hscTnI >100% after ECT compared to baseline with at least one value above the limit of quantification (10 ng/L). 12-lead ECG and hscTnI values were obtained prior to and 15–30 minutes after ECT; in a subset of patients an additional 2-hour hscTnI value was obtained. Results The final study population was 100 patients and a total of 245 ECT treatment sessions. Eight patients (8/100, 8%) experienced new hscTnI elevation after ECT with a cumulative incidence of 3.7% (9/245 treatments; one patient had two hscTnI elevations), two of whom had a non-ST-elevation myocardial infarction (incidence 2/245, 0.8%). Median hscTnI concentrations did not increase significantly after ECT. Tachycardia and/or elevated systolic blood pressure developed after approximately two thirds of ECT treatments. Conclusions ECT appears safe from a cardiac standpoint in a large majority of patients. A small subset of patients with pre-existing cardiovascular risk factors, however, may develop new cardiac troponin elevation after ECT, the clinical relevance of which is unclear in the absence of signs of myocardial ischemia. PMID:28166110

  8. High sensitivity pyrogen testing in water and dialysis solutions.

    Science.gov (United States)

    Daneshian, Mardas; Wendel, Albrecht; Hartung, Thomas; von Aulock, Sonja

    2008-07-20

    The dialysis patient is confronted with hundreds of litres of dialysis solution per week, which pass the natural protective barriers of the body and are brought into contact with the tissue directly in the case of peritoneal dialysis or indirectly in the case of renal dialysis (hemodialysis). The components can be tested for living specimens or dead pyrogenic (fever-inducing) contaminations. The former is usually detected by cultivation and the latter by the endotoxin-specific Limulus Amoebocyte Lysate Assay (LAL). However, the LAL assay does not reflect the response of the human immune system to the wide variety of possible pyrogenic contaminations in dialysis fluids. Furthermore, the test is limited in its sensitivity to detect extremely low concentrations of pyrogens, which in their sum result in chronic pathologies in dialysis patients. The In vitro Pyrogen Test (IPT) employs human whole blood to detect the spectrum of pyrogens to which humans respond by measuring the release of the endogenous fever mediator interleukin-1beta. Spike recovery checks exclude interference. The test has been validated in an international study for pyrogen detection in injectable solutions. In this study we adapted the IPT to the testing of dialysis solutions. Preincubation of 50 ml spiked samples with albumin-coated microspheres enhanced the sensitivity of the assay to detect contaminations down to 0.1 pg/ml LPS or 0.001 EU/ml in water or saline and allowed pyrogen detection in dialysis concentrates or final working solutions. This method offers high sensitivity detection of human-relevant pyrogens in dialysis solutions and components.

  9. Lasers technology

    International Nuclear Information System (INIS)

    2014-01-01

    The Laser Technology Program of IPEN is developed by the Center for Lasers and Applications (CLA) and is committed to the development of new lasers based on the research of new optical materials and new resonator technologies. Laser applications and research occur within several areas such as Nuclear, Medicine, Dentistry, Industry, Environment and Advanced Research. Additional goals of the Program are human resource development and innovation, in association with Brazilian Universities and commercial partners

  10. 5.5 W near-diffraction-limited power from resonant leaky-wave coupled phase-locked arrays of quantum cascade lasers

    International Nuclear Information System (INIS)

    Kirch, J. D.; Chang, C.-C.; Boyle, C.; Mawst, L. J.; Botez, D.; Lindberg, D.; Earles, T.

    2015-01-01

    Five, 8.36 μm-emitting quantum-cascade lasers (QCLs) have been monolithically phase-locked in the in-phase array mode via resonant leaky-wave coupling. The structure is fabricated by etch and regrowth which provides large index steps (Δn = 0.10) between antiguided-array elements and interelement regions. Such high index contrast photonic-crystal (PC) lasers have more than an order of magnitude higher index contrast than PC-distributed feedback lasers previously used for coherent beam combining in QCLs. Absorption loss to metal layers inserted in the interelement regions provides a wide (∼1.0 μm) range in interelement width over which the resonant in-phase mode is strongly favored to lase. Room-temperature, in-phase-mode operation with ∼2.2 kA/cm 2 threshold-current density is obtained from 105 μm-wide aperture devices. The far-field beam pattern has lobewidths 1.65× diffraction limit (D.L.) and 82% of the light in the main lobe, up to 1.8× threshold. Peak pulsed near-D.L. power of 5.5 W is obtained, with 4.5 W emitted in the main lobe. Means of how to increase the device internal efficiency are discussed

  11. Investigation of change of tumor optical properties after laser-induced plasmon-resonant photothermal treatment of transplanted tumors in rats

    Science.gov (United States)

    Genin, Vadim D.; Genina, Elina A.; Bucharskaya, Alla B.; Tuchin, Valery V.; Khlebtsov, Nikolay G.; Terentyuk, Georgy S.; Bashkatov, Alexey N.

    2018-04-01

    The paper presents the investigation of change of tumor optical properties of the rat tumor doped by gold nanoparticles after laser-induced plasmon-resonant photothermal treatment. To obtain the model tumors the rats have been implanted by suspension of alveolar kidney cancer cells. An hour before the experiment the animals have been injected by the suspension of gold nanorods intratumorally. For irradiation a diode laser with wavelength 808 nm has been used. After the irradiation the tumor has been removed and sliced. Spectra of total and collimated transmission and diffuse reflectance of the samples of different layers of the tumors have been measured in the wavelength range 350-2500 nm. Absorption, scattering, reduced scattering coefficients and scattering anisotropy factor of tumor tissues have been calculated with inverse adding-doubling method. The results of the experiment have shown that after doping the tumor tissue by the plasmon resonant nanoparticles and NIR laser irradiating, there is the decreases of absorption as well as scattering properties of the tumor and surrounding tissues. However, despite the sufficiently high temperature on the surface (about 80°C), the changes in the center of the tumor are insignificant.

  12. Two methods for nuclear spin determination in collinear laser spectroscopy: classical r.f. magnetic resonance and observation of the Larmor precession

    International Nuclear Information System (INIS)

    Bendali, N.; Duong, H.T.; Saint-Jalm, J.M.; Vialle, J.L.

    1984-01-01

    Measurement of nuclear spin in the collinear laser spectroscopy method has been investigated using a fast sodium atomic beam excited collinearly by a C.W. single mode dye laser beam. The atomic magnetic moments are first aligned by optical pumping process, then they interact with a static magnetic field H 0 . The magnetic alignment of the atomic system just at the exit of the magnetic field is monitored by the laser induced fluorescence. Upon varying the amplitude of H 0 , the fluorescence signal presents a fringed structure. This structure is due to the Larmor precession of the aligned magnetic moments around H 0 , and therefore it is a signature of the spin involved. The modulation patterns corresponding to different relative orientations of H 0 and light polarization direction, are fitted by an analytical formula. In a second step, a classical magnetic resonance experiment with a static magnetic field and a radiofrequency field has been performed. The monocinetic character of our fast atomic beam allowed us to observe, even at high r.f. power, resonances line shapes in agreement with the Majorana formula

  13. Fabrication and Characterization of High-Sensitivity Underwater Acoustic Multimedia Communication Devices with Thick Composite PZT Films

    Directory of Open Access Journals (Sweden)

    Jeng-Cheng Liu

    2017-01-01

    Full Text Available This paper presents a high-sensitivity hydrophone fabricated with a Microelectromechanical Systems (MEMS process using epitaxial thin films grown on silicon wafers. The evaluated resonant frequency was calculated through finite-element analysis (FEA. The hydrophone was designed, fabricated, and characterized by different measurements performed in a water tank, by using a pulsed sound technique with a sensitivity of −190 dB ± 2 dB for frequencies in the range 50–500 Hz. These results indicate the high-performance miniaturized acoustic devices, which can impact a variety of technological applications.

  14. Introducing wet aerosols into the static high sensitivity ICP (SHIP)

    Energy Technology Data Exchange (ETDEWEB)

    Scheffer, Andy; Engelhard, Carsten; Sperling, Michael; Buscher, Wolfgang [University of Muenster, Institute of Inorganic and Analytical Chemistry, Muenster (Germany)

    2007-08-15

    A demountable design of the static high sensitivity ICP (SHIP) for optical emission spectrometry is presented, and its use as an excitation source with the introduction of wet aerosols was investigated. Aerosols were produced by standard pneumatic sample introduction systems, namely a cross flow nebulizer, Meinhard nebulizer and PFA low flow nebulizer, which have been applied in conjunction with a double pass and a cyclonic spray chamber. The analytical capabilities of these sample introduction systems in combination with the SHIP system were evaluated with respect to the achieved sensitivity. It was found that a nebulizer tailored for low argon flow rates (0.3-0.5 L min{sup -1}) is best suited for the low flow plasma (SHIP). An optimization of all gas flow rates of the SHIP system with the PFA low flow nebulizer was carried out in a two-dimensional way with the signal to background ratio (SBR) and the robustness as optimization target parameters. Optimum conditions for a torch model with 1-mm injector tube were 0.25 and 0.36 L min{sup -1} for the plasma gas and the nebulizer gas, respectively. A torch model with a 2-mm injector tube was optimized to 0.4 L min{sup -1} for the plasma gas and 0.44 L min{sup -1} for the nebulizer gas. In both cases the SHIP system saves approximately 95% of the argon consumed by conventional inductively coupled plasma systems. The limits of detection were found to be in the low microgram per litre range and below for many elements, which was quite comparable to those of the conventional setup. Furthermore, the short-term stability and the wash out behaviour of the SHIP were investigated. Direct comparison with the conventional setup indicated that no remarkable memory effects were caused by the closed design of the torch. The analysis of a NIST SRM 1643e (Trace Elements in Water) with the SHIP yielded recoveries of 97-103% for 13 elements, measured simultaneously. (orig.)

  15. Metal ion-organic compound for high sensitive ESR dosimetry

    International Nuclear Information System (INIS)

    Hassan, G.M.; Ikeya, Motoji

    2000-01-01

    A systematic study to find a tissue equivalent and high sensitive dosimeter material has been made to stimulate the field of ESR dosimetry. Lithium acetate dihydrate (Li-Ac·2H 2 O:CH 3 COOLi·2H 2 O) and lithium phosphate (Li-phosphate:Li 3 PO 4 ) were irradiated by γ-rays to study radicals with (ESR) in addition to magnesium lactate (Mg-lactate (CH 3 CH(OH)COO) 2 Mg) doped with nominal pure lithium lactate (Mg(Li)-lactate) and lithium lactate (CH 3 CH(OH)COOLi) doped with Mg-lactate (Li(Mg)-lactate). A triplet spectrum with intensity ratio of 1:2:1 in Li-Ac·2H 2 O was ascribed to acetate radical which has g=2.0031±0.0004 and hyperfine splitting of A/gβ=2.12±0.1 mT. The Li-phosphate spectrum shows splitting due to anisotropic g-factors of g par =2.0190±0.0005 and g perp =1.9974±0.0004. Quartet spectra with the intensity ratio of 1:3:3:1 in Mg(Li)-lactate and Li(Mg)-lactate were ascribed to lactate radicals with g-factors of 2.0032 ± 0.0004 and 2.0029 ± 0.0004 and the intensity ratio of 1:3:3:1 and A/gβ=1.92±0.06 and 1.82 ± 0.06 mT, respectively. The response to γ-ray dose and the thermal stability as well as the effect of UV-illumination have been studied. The obtained number of free radicals per 100 eV (G-values) were 0.4 ± 0.13, 1.02 ± 0.31, 1.35 ± 0.35 and 0.78 ± 0 for Li-Ac.2H 2 O, Li-phosphate, Mg(Li)-lactate, and Li(Mg)-lactate, respectively. The lifetimes were estimated from Arrhenius plots to be approximately 2.0 ± 0.6, 50.7 ± 20 and 10 ± 3.5 years for Li-phosphate, Mg(Li)-lactate and Li(Mg)-lactate, respectively. The lifetime for Li-Ac·2H 2 O cannot be estimated because of the decomposition by heating

  16. Highly sensitive straightness measurement system using a ball-lens

    International Nuclear Information System (INIS)

    Lee, Minho; Yang, Hyun-Ik; Cho, Nahm-Gyoo

    2016-01-01

    In this paper, a new and simple optical technique to accurately measure the straightness errors of a linear stage is proposed. To improve the performance, including the measurement sensitivity and resolution of the measurement system, and to simultaneously measure two-dimensional straightness errors (2D straightness errors), an optical system was designed using a laser, a retro-reflector, a ball-lens, and a two-dimensional position sensitive detector (2D PSD). The characteristics of the measurement system were analytically and experimentally investigated. A prototype measurement system was manufactured based on the investigated results, and the performances of this system have been tested. The measuring performance of the system was easily improved by about 12 times using the proposed technique and it can be further improved. It is shown that the proposed technique can easily and effectively improve the performance of a conventional straightness measurement system based on the geometric optical method using a PSD. (paper)

  17. Highly Sensitive Cadmium Concentration Sensor Using Long Period Grating

    Directory of Open Access Journals (Sweden)

    A. S. Lalasangi

    2011-08-01

    Full Text Available In this paper we have proposed a simple and effective Long Period Grating chemical sensor for detecting the traces of Cadmium (Cd++ in drinking water at ppm level. Long Period gratings (LPG were fabricated by point-by-point technique with CO2 laser. We have characterized the LPG concentration sensor sensitivity for different solutions of Cd concentrations varying from 0.01 ppm to 0.04 ppm by injecting white Light source and observed transmitted spectra using Optical Spectrum Analyzer (OSA. Proper reagents have been used in the solutions for detection of the Cd species. The overall shift in wavelength is 10 nm when surrounding medium gradually changed from water to 0.04 ppm of cadmium concentrations. A comparative study has been done using sophisticated spectroscopic atomic absorption spectrometer (AAS and Inductively Coupled Plasma (ICP instruments. The spectral sensitivity enhancement was done by modifying grating surface with gold nanoparticles.

  18. A new compact, high sensitivity neutron imaging system

    Energy Technology Data Exchange (ETDEWEB)

    Caillaud, T.; Landoas, O.; Briat, M.; Rosse, B.; Thfoin, I.; Philippe, F.; Casner, A.; Bourgade, J. L.; Disdier, L. [CEA, DAM, DIF,F-91297 Arpajon (France); Glebov, V. Yu.; Marshall, F. J.; Sangster, T. C. [Laboratory for Laser Energetics, University of Rochester, 250 East River Road, Rochester, New York 14623-1299 (United States); Park, H. S.; Robey, H. F.; Amendt, P. [Lawrence Livermore National Laboratory, Livermore, California 94550 (United States)

    2012-10-15

    We have developed a new small neutron imaging system (SNIS) diagnostic for the OMEGA laser facility. The SNIS uses a penumbral coded aperture and has been designed to record images from low yield (10{sup 9}-10{sup 10} neutrons) implosions such as those using deuterium as the fuel. This camera was tested at OMEGA in 2009 on a rugby hohlraum energetics experiment where it recorded an image at a yield of 1.4 Multiplication-Sign 10{sup 10}. The resolution of this image was 54 {mu}m and the camera was located only 4 meters from target chamber centre. We recently improved the instrument by adding a cooled CCD camera. The sensitivity of the new camera has been fully characterized using a linear accelerator and a {sup 60}Co {gamma}-ray source. The calibration showed that the signal-to-noise ratio could be improved by using raw binning detection.

  19. A new compact, high sensitivity neutron imaging system

    International Nuclear Information System (INIS)

    Caillaud, T.; Landoas, O.; Briat, M.; Rossé, B.; Thfoin, I.; Philippe, F.; Casner, A.; Bourgade, J. L.; Disdier, L.; Glebov, V. Yu.; Marshall, F. J.; Sangster, T. C.; Park, H. S.; Robey, H. F.; Amendt, P.

    2012-01-01

    We have developed a new small neutron imaging system (SNIS) diagnostic for the OMEGA laser facility. The SNIS uses a penumbral coded aperture and has been designed to record images from low yield (10 9 –10 10 neutrons) implosions such as those using deuterium as the fuel. This camera was tested at OMEGA in 2009 on a rugby hohlraum energetics experiment where it recorded an image at a yield of 1.4 × 10 10 . The resolution of this image was 54 μm and the camera was located only 4 meters from target chamber centre. We recently improved the instrument by adding a cooled CCD camera. The sensitivity of the new camera has been fully characterized using a linear accelerator and a 60 Co γ-ray source. The calibration showed that the signal-to-noise ratio could be improved by using raw binning detection.

  20. A High Sensitivity EPR Technique for Alanine Dosimetry (invited paper)

    International Nuclear Information System (INIS)

    Haskell, E.H.; Hayes, R.B.; Kenner, G.H.

    1998-01-01

    Uncertainties of ± 5 mGy were achieved in the measurement of alanine dosemeters using optimised EPR parameters, instrumentation, spectral manipulation and subtraction techniques. Modulation amplitude and microwave power were adjusted to combine resonances of two neighbouring alanine signals. Instrumental variations were minimised by combining and subtracting pre- and post-measurement spectra of the empty EPR tube. A spectrum of the native signal of non-dosed alanine was generated from a single batch of dosemeters and subtracted from spectra of the irradiated dosemeters, also from the same batch. Field alignment was adjusted with the use of an in-cavity Mn ++ standard. A constant rotation goniometer was used to eliminate anisotropies in the EPR tube and alanine samples. Finally, digital filters were applied to the resulting spectra. (author)

  1. Design of 1+ Ion Source Coupling First Design of the Resonant Ionization Laser Ion Source For the Multi-Mega Watt Target Station

    CERN Document Server

    A. Olivier-Kaiser, F. Le Blanc, C. Lau

    The realisation of next-generation ion sources suitable for the EURISOL multi-mega-watt (MMW) target station needs exhaustive studies and developments. An exhaustive review was carried out to evaluate the capability of the ion-sources to operate under the irradiation conditions of the MMW target station. In addition, selectivity must be taken into account to avoid the spread of unwanted radioactivity out of the target-ion-source system (TIS).These studies led to consider RILIS (Resonance Ionization Laser Ion Source) as the reference ion source for this target station.

  2. Hyperfine structure of the X 2Σ+ ground state of Ca 35Cl and Ca 37Cl by molecular-beam, laser-rf double resonance

    International Nuclear Information System (INIS)

    Childs, W.J.; Cok, D.R.; Goodman, L.S.

    1982-01-01

    The hyperfine structure of the X 2 Σ + state of Ca 35 Cl and Ca 37 Cl, unresolved in previous studies, has been investigated in detail by the molecular-beam, laser-rf, double-resonance technique. Results for the spin-rotation interaction and the dipole and quadrupole hfs constants are given in the form of Dunham coefficients so that the N'' and v'' dependence of each constant can be explicitly exhibited. The results, after dividing out the purely nuclear effects, fall between the corresponding values for CaF and CaBr, as expected

  3. $\\beta$-decay study of neutron-rich Tl, Pb, and Bi by means of the pulsed-release technique and resonant laser ionisation

    CERN Multimedia

    Lettry, J

    2002-01-01

    It is proposed to study new neutron-rich nuclei around the Z = 82 magic shell closure, with major relevance for understanding the evolution of nuclear structure at extreme isospin values. Following the IS354 experiment, $\\beta$-decay studies of neutron-rich thallium, lead and bismuth isotopes will be performed for 215 $\\leqslant$ A $\\leqslant$ 219. To this purpose the pulsed-release technique, which was pioneered at ISOLDE, will be optimised. It will be complemented with the higher element selectivity that can be obtained by the unique features of resonant laser ionisation, available at ISOLDE from the RILIS source.

  4. The observation of the Ne-like ion resonance line satellites for CrXV ... Ni XIX CO2-laser produced plasma

    International Nuclear Information System (INIS)

    Khakhalin, S.Ya.; Faenov, A.Ya.; Skobelev, I.Yu.; Pikuz, S.A.; Nilsen, J.; Osterheld, A.

    1994-01-01

    We present an analysis of dielectronic satellite spectra of Ne-like ion resonance lines for elements from Cr to Ni. For these low-Z elements, we use spectra from strongly underionized CO 2 -laser produced plasma to minimize the emission from open L-shell ions. This simplifies the spectra and allows the identification of satellite lines caused by radiative transitions from autoionizing states of sodium like ions. Good agreement between the satellite structure calculations and the experimental emission spectra is obtained. (orig.)

  5. The observation of the Ne-like ion resonance line satellites for CrXV. Ni XIX CO[sub 2]-laser produced plasma

    Energy Technology Data Exchange (ETDEWEB)

    Khakhalin, S.Ya. (MISDC, NPO ' ' VNIIFTRI' ' , Mendeleevo (Russian Federation)); Faenov, A.Ya. (MISDC, NPO ' ' VNIIFTRI' ' , Mendeleevo (Russian Federation)); Skobelev, I.Yu. (MISDC, NPO ' ' VNIIFTRI' ' , Mendeleevo (Russian Federation)); Pikuz, S.A. (P. N. Lebedev Physical Inst., Russian Academy of Science, Moscow (Russian Federation)); Nilsen, J. (Lawrence Livermore National Lab., Livermore, CA (United States)); Osterheld, A. (Lawrence Livermore National Lab., Livermore, CA (United States))

    1994-08-01

    We present an analysis of dielectronic satellite spectra of Ne-like ion resonance lines for elements from Cr to Ni. For these low-Z elements, we use spectra from strongly underionized CO[sub 2]-laser produced plasma to minimize the emission from open L-shell ions. This simplifies the spectra and allows the identification of satellite lines caused by radiative transitions from autoionizing states of sodium like ions. Good agreement between the satellite structure calculations and the experimental emission spectra is obtained. (orig.).

  6. A surface acoustic wave humidity sensor with high sensitivity based on electrospun MWCNT/Nafion nanofiber films

    International Nuclear Information System (INIS)

    Lei Sheng; Chen Dajing; Chen Yuquan

    2011-01-01

    Humidity detection has been widely used in a variety of fields. A humidity sensor with high sensitivity is reported in this paper. A surface acoustic wave resonator (SAWR) with high resonance frequency was fabricated as a basic sensitive component. Various nanotechnologies were used to improve the sensor's performance. A multi-walled carbon nanotube/Nafion (MWCNT/Nafion) composite material was prepared as humidity-sensitive films, deposited on the surface of an SAWR by the electrospinning method. The electrospun MWCNT/Nafion nanofiber films showed a three-dimensional (3D) porous structure, which was profitable for improving the sensor's performance. The new nano-water-channel model of Nafion was also applied in the humidity sensing process. Compared to other research, the present sensor showed excellent sensitivity (above 400 kHz/% relative humidity (RH) in the range from 10% RH to 80% RH), good linearity (R 2 > 0.98) and a short response time (∼3 s-63%).

  7. New application of superconductors: High sensitivity cryogenic light detectors

    Energy Technology Data Exchange (ETDEWEB)

    Cardani, L., E-mail: laura.cardani@roma1.infn.it [Dipartimento di Fisica, Sapienza Università di Roma, Piazzale Aldo Moro 2, 00185 Roma (Italy); Physics Department, Princeton University, Washington Road, 08544 Princeton, NJ (United States); Bellini, F.; Casali, N. [Dipartimento di Fisica, Sapienza Università di Roma, Piazzale Aldo Moro 2, 00185 Roma (Italy); INFN – Sezione di Roma, Piazzale Aldo Moro 2, 00185 Roma, Italy (Italy); Castellano, M.G. [Istituto di Fotonica e Nanotecnologie – CNR, Via Cineto Romano 42, 00156 Roma (Italy); Colantoni, I.; Coppolecchia, A. [Dipartimento di Fisica, Sapienza Università di Roma, Piazzale Aldo Moro 2, 00185 Roma (Italy); Cosmelli, C.; Cruciani, A. [Dipartimento di Fisica, Sapienza Università di Roma, Piazzale Aldo Moro 2, 00185 Roma (Italy); INFN – Sezione di Roma, Piazzale Aldo Moro 2, 00185 Roma, Italy (Italy); D' Addabbo, A. [INFN – Laboratori Nazionali del Gran Sasso, Assergi (L' Aquila) 67010 (Italy); Di Domizio, S. [INFN – Sezione di Genova, Via Dodecaneso 33, 16146 Genova (Italy); Dipartimento di Fisica, Università degli Studi di Genova, Via Dodecaneso 33, 16146 Genova (Italy); Martinez, M. [Dipartimento di Fisica, Sapienza Università di Roma, Piazzale Aldo Moro 2, 00185 Roma (Italy); INFN – Sezione di Roma, Piazzale Aldo Moro 2, 00185 Roma, Italy (Italy); Laboratorio de Fisica Nuclear y Astroparticulas, Universidad de Zaragoza, Zaragoza 50009 (Spain); Tomei, C. [INFN – Sezione di Roma, Piazzale Aldo Moro 2, 00185 Roma, Italy (Italy); and others

    2017-02-11

    In this paper we describe the current status of the CALDER project, which is developing ultra-sensitive light detectors based on superconductors for cryogenic applications. When we apply an AC current to a superconductor, the Cooper pairs oscillate and acquire kinetic inductance, that can be measured by inserting the superconductor in a LC circuit with high merit factor. Interactions in the superconductor can break the Cooper pairs, causing sizable variations in the kinetic inductance and, thus, in the response of the LC circuit. The continuous monitoring of the amplitude and frequency modulation allows to reconstruct the incident energy with excellent sensitivity. This concept is at the basis of Kinetic Inductance Detectors (KIDs) that are characterized by natural aptitude to multiplexed read-out (several sensors can be tuned to different resonant frequencies and coupled to the same line), resolution of few eV, stable behavior over a wide temperature range, and ease in fabrication. We present the results obtained by the CALDER collaboration with 2×2 cm{sup 2} substrates sampled by 1 or 4 Aluminum KIDs. We show that the performances of the first prototypes are already competitive with those of other commonly used light detectors, and we discuss the strategies for a further improvement.

  8. New application of superconductors: High sensitivity cryogenic light detectors

    International Nuclear Information System (INIS)

    Cardani, L.; Bellini, F.; Casali, N.; Castellano, M.G.; Colantoni, I.; Coppolecchia, A.; Cosmelli, C.; Cruciani, A.; D'Addabbo, A.; Di Domizio, S.; Martinez, M.; Tomei, C.

    2017-01-01

    In this paper we describe the current status of the CALDER project, which is developing ultra-sensitive light detectors based on superconductors for cryogenic applications. When we apply an AC current to a superconductor, the Cooper pairs oscillate and acquire kinetic inductance, that can be measured by inserting the superconductor in a LC circuit with high merit factor. Interactions in the superconductor can break the Cooper pairs, causing sizable variations in the kinetic inductance and, thus, in the response of the LC circuit. The continuous monitoring of the amplitude and frequency modulation allows to reconstruct the incident energy with excellent sensitivity. This concept is at the basis of Kinetic Inductance Detectors (KIDs) that are characterized by natural aptitude to multiplexed read-out (several sensors can be tuned to different resonant frequencies and coupled to the same line), resolution of few eV, stable behavior over a wide temperature range, and ease in fabrication. We present the results obtained by the CALDER collaboration with 2×2 cm"2 substrates sampled by 1 or 4 Aluminum KIDs. We show that the performances of the first prototypes are already competitive with those of other commonly used light detectors, and we discuss the strategies for a further improvement.

  9. Ultra-high sensitivity imaging of cancer using SERRS nanoparticles

    Science.gov (United States)

    Kircher, Moritz F.

    2016-05-01

    "Surface-enhanced Raman spectroscopy" (SERS) nanoparticles have gained much attention in recent years for in silico, in vitro and in vivo sensing applications. Our group has developed novel generations of biocompatible "surfaceenhanced resonance Raman spectroscopy" (SERRS) nanoparticles as novel molecular imaging agents. Via rigorous optimization of the different variables contributing to the Raman enhancement, we were able to design SERRS nanoparticles with so far unprecedented sensitivity of detection under in vivo imaging conditions (femto-attomolar range). This has resulted in our ability to visualize, with a single nanoparticle, many different cancer types (after intravenous injection) in mouse models. The cancer types we have tested so far include brain, breast, esophagus, stomach, pancreas, colon, sarcoma, and prostate cancer. All mouse models used are state-of-the-art and closely mimic the tumor biology in their human counterparts. In these animals, we were able to visualize not only the bulk tumors, but importantly also microscopic extensions and locoregional satellite metastases, thus delineating for the first time the true extent of tumor spread. Moreover, the particles enable the detection of premalignant lesions. Given their inert composition they are expected to have a high chance for clinical translation, where we envision them to have an impact in various scenarios ranging from early detection, image-guidance in open or minimally invasive surgical procedures, to noninvasive imaging in conjunction with spatially offset (SESORS) Raman detection devices.

  10. Laser induced fluorescence spectroscopy in atomic beams of radioactive nuclides

    International Nuclear Information System (INIS)

    Rebel, H.; Schatz, G.

    1982-01-01

    Measurements of the resonant scattering of light from CW tunable dye lasers, by a well collimated atomic beam, enable hyperfine splittings and optical isotope shifts to be determined with high precision and high sensitivity. Recent off-line atomic beam experiments with minute samples, comprising measurements with stable and unstable Ba, Ca and Pb isotopes are reviewed. The experimental methods and the analysis of the data are discussed. Information on the variation of the rms charge radii and on electromagnetic moments of nuclei in long isotopic chains is presented. (orig.) [de

  11. Highly Sensitive DNA Sensor Based on Upconversion Nanoparticles and Graphene Oxide.

    Science.gov (United States)

    Alonso-Cristobal, P; Vilela, P; El-Sagheer, A; Lopez-Cabarcos, E; Brown, T; Muskens, O L; Rubio-Retama, J; Kanaras, A G

    2015-06-17

    In this work we demonstrate a DNA biosensor based on fluorescence resonance energy transfer (FRET) between NaYF4:Yb,Er nanoparticles and graphene oxide (GO). Monodisperse NaYF4:Yb,Er nanoparticles with a mean diameter of 29.1 ± 2.2 nm were synthesized and coated with a SiO2 shell of 11 nm, which allowed the attachment of single strands of DNA. When these DNA-functionalized NaYF4:Yb,Er@SiO2 nanoparticles were in the proximity of the GO surface, the π-π stacking interaction between the nucleobases of the DNA and the sp(2) carbons of the GO induced a FRET fluorescence quenching due to the overlap of the fluorescence emission of the NaYF4:Yb,Er@SiO2 and the absorption spectrum of GO. By contrast, in the presence of the complementary DNA strands, the hybridization leads to double-stranded DNA that does not interact with the GO surface, and thus the NaYF4:Yb,Er@SiO2 nanoparticles remain unquenched and fluorescent. The high sensitivity and specificity of this sensor introduces a new method for the detection of DNA with a detection limit of 5 pM.

  12. Highly sensitive detection of molecular interactions with plasmonic optical fiber grating sensors.

    Science.gov (United States)

    Voisin, Valérie; Pilate, Julie; Damman, Pascal; Mégret, Patrice; Caucheteur, Christophe

    2014-01-15

    Surface Plasmon resonance (SPR) optical fiber biosensors constitute a miniaturized counterpart to the bulky prism configuration and offer remote operation in very small volumes of analyte. They are a cost-effective and relatively straightforward technique to yield in situ (or even possibly in vivo) molecular detection. The biosensor configuration reported in this work uses nanometric-scale gold-coated tilted fiber Bragg gratings (TFBGs) interrogated by light polarized radially to the optical fiber outer surface, so as to maximize the optical coupling with the SPR. These gratings were recently associated to aptamers to assess their label-free biorecognition capability in buffer and serum solutions. In this work, using the well-acknowledged biotin-streptavidin pair as a benchmark, we go forward in the demonstration of their unique sensitivity. In addition to the monitoring of the self-assembled monolayer (SAM) in real time, we report an unprecedented limit of detection (LOD) as low as 2 pM. Finally, an immunosensing experiment is realized with human transferrin (dissociation constant Kd~10(-8) M(-1)). It allows to assess both the reversibility and the robustness of the SPR-TFBG biosensors and to confirm their high sensitivity. © 2013 Published by Elsevier B.V.

  13. Multi-service highly sensitive rectifier for enhanced RF energy scavenging.

    Science.gov (United States)

    Shariati, Negin; Rowe, Wayne S T; Scott, James R; Ghorbani, Kamran

    2015-05-07

    Due to the growing implications of energy costs and carbon footprints, the need to adopt inexpensive, green energy harvesting strategies are of paramount importance for the long-term conservation of the environment and the global economy. To address this, the feasibility of harvesting low power density ambient RF energy simultaneously from multiple sources is examined. A high efficiency multi-resonant rectifier is proposed, which operates at two frequency bands (478-496 and 852-869 MHz) and exhibits favorable impedance matching over a broad input power range (-40 to -10 dBm). Simulation and experimental results of input reflection coefficient and rectified output power are in excellent agreement, demonstrating the usefulness of this innovative low-power rectification technique. Measurement results indicate an effective efficiency of 54.3%, and an output DC voltage of 772.8 mV is achieved for a multi-tone input power of -10 dBm. Furthermore, the measured output DC power from harvesting RF energy from multiple services concurrently exhibits a 3.14 and 7.24 fold increase over single frequency rectification at 490 and 860 MHz respectively. Therefore, the proposed multi-service highly sensitive rectifier is a promising technique for providing a sustainable energy source for low power applications in urban environments.

  14. High sensitive photonic crystal multiplexed biosensor array using H0 sandwiched cavities

    Directory of Open Access Journals (Sweden)

    Arafa Safia

    2017-01-01

    Full Text Available We theoretically investigate a high sensitive photonic crystal integrated biosensor array structure which is potentially used for label-free multiplexed sensing. The proposed device consists of an array of three sandwiched H0 cavities patterned above silicon on insulator (SOI substrate; each cavity has been designed for different cavity spacing and different resonant wavelength. Results obtained by performing finite-difference time-domain (FDTD simulations, indicate that the response of each detection unit shifts independently in terms of refractive index variations. The optimized design makes possible the combination of sensing as a function of location, as well as a function of time in the same platform. A refractive index sensitivity of 520nm/RIU and a quality factor over 104 are both achieved with an accompanied crosstalk of less than -26 dB. In addition, the device presents an improved detection limit (DL of 1.24.10-6 RIU and a wide measurement range. These features make the designed device a promising element for performing label-free multiplexed detection in monolithic substrate for medical diagnostics and environmental monitoring.

  15. No-core fiber-based highly sensitive optical fiber pH sensor.

    Science.gov (United States)

    Bhardwaj, Vanita; Pathak, Akhilesh Kumar; Singh, Vinod Kumar

    2017-05-01

    The present work describes the fabrication and characterization of an optical fiber pH sensor using a sol–gel technique. The sensing head configuration is incorporated using a short section of no-core fiber, coated with tetraethyl orthosilicate and spliced at the end of a single mode fiber with a bulge. Different types of indicators (bromophenol blue, cresol red, and chlorophenol red) were used to achieve a wide pH range from 2 to 13. High sensitivities of the fabricated device were found to be 1.02 and ? 0.93 ?? nm / pH for acidic and alkaline solutions, respectively. From the characterization results, it was noted that there is an impact of ionic strength and an effect of the temperature of liquid on the response characteristic, which is an advantage of the existing device over the other pH sensors. The fabricated sensor exhibited good reflection spectrum, indicating a blueshift in resonance wavelength for alkaline solutions and a redshift for acidic solutions.

  16. High-Sensitivity Troponin: A Clinical Blood Biomarker for Staging Cardiomyopathy in Fabry Disease.

    Science.gov (United States)

    Seydelmann, Nora; Liu, Dan; Krämer, Johannes; Drechsler, Christiane; Hu, Kai; Nordbeck, Peter; Schneider, Andreas; Störk, Stefan; Bijnens, Bart; Ertl, Georg; Wanner, Christoph; Weidemann, Frank

    2016-05-31

    High-sensitivity troponin (hs-TNT), a biomarker of myocardial damage, might be useful for assessing fibrosis in Fabry cardiomyopathy. We performed a prospective analysis of hs-TNT as a biomarker for myocardial changes in Fabry patients and a retrospective longitudinal follow-up study to assess longitudinal hs-TNT changes relative to fibrosis and cardiomyopathy progression. For the prospective analysis, hs-TNT from 75 consecutive patients with genetically confirmed Fabry disease was analyzed relative to typical Fabry-associated echocardiographic findings and total myocardial fibrosis as measured by late gadolinium enhancement (LE) on magnetic resonance imaging. Longitudinal data (3.9±2.0 years), including hs-TNT, LE, and echocardiographic findings from 58 Fabry patients, were retrospectively collected. Hs-TNT level positively correlated with LE (linear correlation coefficient, 0.72; odds ratio, 32.81 [95% CI, 3.56-302.59]; P=0.002); patients with elevated baseline hs-TNT (>14 ng/L) showed significantly increased LE (median: baseline, 1.9 [1.1-3.3] %; follow-up, 3.2 [2.3-4.9] %; PFabry disease and a qualified predictor of cardiomyopathy progression. Thus, hs-TNT could be helpful for staging and follow-up of Fabry patients. © 2016 The Authors. Published on behalf of the American Heart Association, Inc., by Wiley Blackwell.

  17. Multi-Service Highly Sensitive Rectifier for Enhanced RF Energy Scavenging

    Science.gov (United States)

    Shariati, Negin; Rowe, Wayne S. T.; Scott, James R.; Ghorbani, Kamran

    2015-01-01

    Due to the growing implications of energy costs and carbon footprints, the need to adopt inexpensive, green energy harvesting strategies are of paramount importance for the long-term conservation of the environment and the global economy. To address this, the feasibility of harvesting low power density ambient RF energy simultaneously from multiple sources is examined. A high efficiency multi-resonant rectifier is proposed, which operates at two frequency bands (478–496 and 852–869 MHz) and exhibits favorable impedance matching over a broad input power range (−40 to −10 dBm). Simulation and experimental results of input reflection coefficient and rectified output power are in excellent agreement, demonstrating the usefulness of this innovative low-power rectification technique. Measurement results indicate an effective efficiency of 54.3%, and an output DC voltage of 772.8 mV is achieved for a multi-tone input power of −10 dBm. Furthermore, the measured output DC power from harvesting RF energy from multiple services concurrently exhibits a 3.14 and 7.24 fold increase over single frequency rectification at 490 and 860 MHz respectively. Therefore, the proposed multi-service highly sensitive rectifier is a promising technique for providing a sustainable energy source for low power applications in urban environments. PMID:25951137

  18. Application of resonance ionization mass spectrometry for trace analysis and in fundamental research

    International Nuclear Information System (INIS)

    Passler, G.

    1997-01-01

    Resonance ionization mass spectrometry (RIMS) has been used for ultra-trace analysis on long-lived radioisotopes like Pu, Tc and 89,90 Sr in various environmental samples. The experimental approaches cover pulsed laser spectroscopy on a thermal atomic beam and subsequent time-of-flight mass analysis, a pulsed laser ion source combined with conventional mass spectrometry, and collinear resonance ionization on a mass-separated fast atomic beam. The high sensitivity of RIMS also enables atomic spectroscopy on rare isotopes. For the first time experimental values for the ionization potential of actinides up to Cf have been determined. The paper reviews the dependency of the different experimental approaches on the analytical problem. copyright 1997 American Institute of Physics

  19. Development of double-pulse lasers ablation system and electron paramagnetic resonance spectroscopy for direct spectral analysis of manganese doped PVA polymer

    Science.gov (United States)

    Khalil, A. A. I.; Morsy, M. A.; El-Deen, H. Z.

    2017-11-01

    Series of manganese-co-precipitated poly (vinyl alcohol) (PVA) polymer were quantitatively and qualitatively analyzed using laser ablation system (LAS) based on double-pulse laser induced breakdown spectroscopy (DP-LIBS) and electron paramagnetic resonance (EPR) spectroscopy. The collinear nanosecond laser beams of 266 and 1064 nm were optimized to focus on the surface of the PVA polymer target. Both laser beams were employed to estimate the natural properties of the excited Mn-PVA plasma, such as electron number density (Ne), electron temperature (Te), and Mn concentration. Individual transition lines of manganese (Mn), carbon (C), lithium (Li), hydrogen (H) and oxygen (O) atoms are identified based on the NIST spectral database. The results show better responses with DP-LIBS than the single-pulse laser induced breakdown spectroscopy (SP-LIBS). On the other hand, the EPR investigation shows characteristic broad peak of Mn-nano-particles (Mn-NPs) in the range of quantum dots of superparamagnetic materials. The line width (peak-to-peak, ΔHpp) and g-value of the observed Mn-EPR peak are ∼20 mT and 2.0046, respectively. The intensities of Mn-emission line at a wavelength 403.07 nm and the Mn-EPR absorption peak were used to accurate quantify the Mn-content in the polymer matrix. The results produce linear trends within the studied concentration range with regression coefficient (R2) value of ∼0.99, and limit of detection (LOD) of 0.026 mol.% and 0.016 mol.%, respectively. The LOD values are at a fold change of about -0.2 of the studied lowest mol.%. The proposed protocols of trace element detection are of significant advantage and can be applied to the other metal analysis.

  20. High-efficiency generation of pulsed Lyman-α radiation by resonant laser wave mixing in low pressure Kr-Ar mixture.

    Science.gov (United States)

    Saito, Norihito; Oishi, Yu; Miyazaki, Koji; Okamura, Kotaro; Nakamura, Jumpei; Louchev, Oleg A; Iwasaki, Masahiko; Wada, Satoshi

    2016-04-04

    We report an experimental generation of ns pulsed 121.568 nm Lyman-α radiation by the resonant nonlinear four-wave mixing of 212.556 nm and 845.015 nm radiation pulses providing a high conversion efficiency 1.7x10-3 with the output pulse energy 3.6 μJ achieved using a low pressure Kr-Ar mixture. Theoretical analysis shows that this efficiency is achieved due to the advantage of using (i) the high input laser intensities in combination with (ii) the low gas pressure allowing us to avoid the onset of full-scale discharge in the laser focus. In particular, under our experimental conditions the main mechanism of photoionization caused by the resonant 2-photon 212.556 nm radiation excitation of Kr atoms followed by the 1-photon ionization leads to ≈17% loss of Kr atoms and efficiency loss only by the end of the pulse. The energy of free electrons, generated by 212.556 nm radiation via (2 + 1)-photon ionization and accelerated mainly by 845.015 nm radiation, remains during the pulse below the level sufficient for the onset of full-scale discharge by the electron avalanche. Our analysis also suggests that ≈30-fold increase of 845.015 nm pulse energy can allow one to scale up the L-α radiation pulse energy towards the level of ≈100 μJ.

  1. Laser Displacement Measurements of Fan Blades in Resonance and Flutter During the Boundary Layer Ingesting Inlet and Distortion-Tolerant Fan Test

    Science.gov (United States)

    Duffy, Kirsten P.; Provenza, Andrew J.; Bakhle, Milind A.; Min, James B.; Abdul-Aziz, Ali

    2018-01-01

    NASA's Advanced Air Transport Technology Project is investigating boundary layer ingesting propulsors for future subsonic commercial aircraft to improve aircraft efficiency, thereby reducing fuel burn. To that end, a boundary layer ingesting inlet and distortion-tolerant fan stage was designed, fabricated, and tested within the 8' x 6' Supersonic Wind Tunnel at NASA Glenn Research Center. Because of the distortion in the air flow over the fan, the blades were designed to withstand a much higher aerodynamic forcing than for a typical clean flow. The blade response for several resonance modes were measured during start-up and shutdown, as well as at near 85% design speed. Flutter in the first bending mode was also observed in the fan at the design speed, at an off-design condition, although instabilities were difficult to instigate with this fan in general. Blade vibrations were monitored through twelve laser displacement probes that were placed around the inner circumference of the casing, at the blade leading and trailing edges. These probes captured the movement of all the blades during the entire test. Results are presented for various resonance mode amplitudes, frequencies and damping, as well as flutter amplitudes and frequency. Benefits and disadvantages of laser displacement probe measurements versus strain gage measurements are discussed.

  2. Resonance laser-plasma excitation of coherent terahertz phonons in the bulk of fluorine-bearing crystals under high-intensity femtosecond laser irradiation

    Energy Technology Data Exchange (ETDEWEB)

    Potemkin, F V; Mareev, E I [International Laser Center, M. V. Lomonosov Moscow State University, Moscow (Russian Federation); Khodakovskii, N G [A M Prokhorov General Physics Institute, Russian Academy of Sciences, Moscow (Russian Federation); Mikheev, P M

    2013-08-31

    The dynamics of coherent phonons in fluorine-containing crystals was investigated by pump-probe technique in the plasma production regime. Several phonon modes, whose frequencies are overtones of the 0.38-THz fundamental frequency, were simultaneously observed in a lithium fluoride crystal. Phonons with frequencies of 1 and 0.1 THz were discovered in a calcium fluoride crystal and coherent phonons with frequencies of 1 THz and 67 GHz were observed in a barium fluoride crystal. Furthermore, in the latter case the amplitudes of phonon mode oscillations were found to significantly increase 15 ps after laser irradiation. (interaction of laser radiation with matter)

  3. A low-noise transimpedance amplifier for the detection of "Violin-Mode" resonances in advanced Laser Interferometer Gravitational wave Observatory suspensions

    Science.gov (United States)

    Lockerbie, N. A.; Tokmakov, K. V.

    2014-11-01

    This paper describes the design and performance of an extremely low-noise differential transimpedance amplifier, which takes its two inputs from separate photodiodes. The amplifier was planned to serve as the front-end electronics for a highly sensitive shadow-displacement sensing system, aimed at detecting very low-level "Violin-Mode" (VM) oscillations in 0.4 mm diameter by 600 mm long fused-silica suspension fibres. Four such highly tensioned fibres support the 40 kg test-masses/mirrors of the Advanced Laser Interferometer Gravitational wave Observatory interferometers. This novel design of amplifier incorporates features which prevent "noise-gain peaking" arising from large area photodiode (and cable) capacitances, and which also usefully separate the DC and AC photocurrents coming from the photodiodes. In consequence, the differential amplifier was able to generate straightforwardly two DC outputs, one per photodiode, as well as a single high-gain output for monitoring the VM oscillations—this output being derived from the difference of the photodiodes' two, naturally anti-phase, AC photocurrents. Following a displacement calibration, the amplifier's final VM signal output was found to have an AC displacement responsivity at 500 Hz of (9.43 ± 1.20) MV(rms) m-1(rms), and, therefore, a shot-noise limited sensitivity to such AC shadow- (i.e., fibre-) displacements of (69 ± 13) picometres/√Hz at this frequency, over a measuring span of ±0.1 mm.

  4. A low-noise transimpedance amplifier for the detection of “Violin-Mode” resonances in advanced Laser Interferometer Gravitational wave Observatory suspensions

    International Nuclear Information System (INIS)

    Lockerbie, N. A.; Tokmakov, K. V.

    2014-01-01

    This paper describes the design and performance of an extremely low-noise differential transimpedance amplifier, which takes its two inputs from separate photodiodes. The amplifier was planned to serve as the front-end electronics for a highly sensitive shadow-displacement sensing system, aimed at detecting very low-level “Violin-Mode” (VM) oscillations in 0.4 mm diameter by 600 mm long fused-silica suspension fibres. Four such highly tensioned fibres support the 40 kg test-masses/mirrors of the Advanced Laser Interferometer Gravitational wave Observatory interferometers. This novel design of amplifier incorporates features which prevent “noise-gain peaking” arising from large area photodiode (and cable) capacitances, and which also usefully separate the DC and AC photocurrents coming from the photodiodes. In consequence, the differential amplifier was able to generate straightforwardly two DC outputs, one per photodiode, as well as a single high-gain output for monitoring the VM oscillations—this output being derived from the difference of the photodiodes’ two, naturally anti-phase, AC photocurrents. Following a displacement calibration, the amplifier's final VM signal output was found to have an AC displacement responsivity at 500 Hz of (9.43 ± 1.20) MV(rms) m −1 (rms), and, therefore, a shot-noise limited sensitivity to such AC shadow- (i.e., fibre-) displacements of (69 ± 13) picometres/√Hz at this frequency, over a measuring span of ±0.1 mm

  5. A low-noise transimpedance amplifier for the detection of "Violin-Mode" resonances in Advanced Laser Interferometer Gravitational wave Observatory suspensions.

    Science.gov (United States)

    Lockerbie, N A; Tokmakov, K V

    2014-11-01

    This paper describes the design and performance of an extremely low-noise differential transimpedance amplifier, which takes its two inputs from separate photodiodes. The amplifier was planned to serve as the front-end electronics for a highly sensitive shadow-displacement sensing system, aimed at detecting very low-level "Violin-Mode" (VM) oscillations in 0.4 mm diameter by 600 mm long fused-silica suspension fibres. Four such highly tensioned fibres support the 40 kg test-masses/mirrors of the Advanced Laser Interferometer Gravitational wave Observatory interferometers. This novel design of amplifier incorporates features which prevent "noise-gain peaking" arising from large area photodiode (and cable) capacitances, and which also usefully separate the DC and AC photocurrents coming from the photodiodes. In consequence, the differential amplifier was able to generate straightforwardly two DC outputs, one per photodiode, as well as a single high-gain output for monitoring the VM oscillations-this output being derived from the difference of the photodiodes' two, naturally anti-phase, AC photocurrents. Following a displacement calibration, the amplifier's final VM signal output was found to have an AC displacement responsivity at 500 Hz of (9.43 ± 1.20) MV(rms) m(-1)(rms), and, therefore, a shot-noise limited sensitivity to such AC shadow- (i.e., fibre-) displacements of (69 ± 13) picometres/√Hz at this frequency, over a measuring span of ±0.1 mm.

  6. Peri-implant osseointegration after low-level laser therapy: micro-computed tomography and resonance frequency analysis in an animal model.

    Science.gov (United States)

    Mayer, Luciano; Gomes, Fernando Vacilotto; de Oliveira, Marília Gerhardt; de Moraes, João Feliz Duarte; Carlsson, Lennart

    2016-12-01

    The purpose of the present study is to evaluate the effects of low-level laser therapy on the osseointegration process by comparing resonance frequency analysis measurements performed at implant placement and after 30 days and micro-computed tomography images in irradiated vs nonirradiated rabbits. Fourteen male New Zealand rabbits were randomly divided into two groups of seven animals each, one control group (nonirradiated animals) and one experimental group that received low-level laser therapy (Thera Lase®, aluminum-gallium-arsenide laser diode, 10 J per spot, two spots per session, seven sessions, 830 nm, 50 mW, CW, Ø 0.0028 cm 2 ). The mandibular left incisor was surgically extracted in all animals, and one osseointegrated implant was placed immediately afterward (3.25ø × 11.5 mm; NanoTite, BIOMET 3i). Resonance frequency analysis was performed with the Osstell® device at implant placement and at 30 days (immediately before euthanasia). Micro-computed tomography analyses were then conducted using a high-resolution scanner (SkyScan 1172 X-ray Micro-CT) to evaluate the amount of newly formed bone around the implants. Irradiated animals showed significantly higher implant stability quotients at 30 days (64.286 ± 1.596; 95 % confidence interval (CI) 60.808-67.764) than controls (56.357 ± 1.596; 95 %CI 52.879-59.835) (P = .000). The percentage of newly formed bone around the implants was also significantly higher in irradiated animals (75.523 ± 8.510; 95 %CI 61.893-89.155) than in controls (55.012 ± 19.840; 95 %CI 41.380-68.643) (P = .027). Laser therapy, based on the irradiation protocol used in this study, was able to provide greater implant stability and increase the volume of peri-implant newly formed bone, indicating that laser irradiation effected an improvement in the osseointegration process.

  7. 110 GHz hybrid mode-locked fiber laser with enhanced extinction ratio based on nonlinear silicon-on-insulator micro-ring-resonator (SOI MRR)

    International Nuclear Information System (INIS)

    Liu, Yang; Hsu, Yung; Chow, Chi-Wai; Yang, Ling-Gang; Lai, Yin-Chieh; Yeh, Chien-Hung; Tsang, Hon-Ki

    2016-01-01

    We propose and experimentally demonstrate a new 110 GHz high-repetition-rate hybrid mode-locked fiber laser using a silicon-on-insulator microring-resonator (SOI MRR) acting as the optical nonlinear element and optical comb filter simultaneously. By incorporating a phase modulator (PM) that is electrically driven at a fraction of the harmonic frequency, an enhanced extinction ratio (ER) of the optical pulses can be produced. The ER of the optical pulse train increases from 3 dB to 10 dB. As the PM is only electrically driven by the signal at a fraction of the harmonic frequency, in this case 22 GHz (110 GHz/5 GHz), a low bandwidth PM and driving circuit can be used. The mode-locked pulse width and the 3 dB spectral bandwidth of the proposed mode-locked fiber laser are measured, showing that the optical pulses are nearly transform limited. Moreover, stability evaluation for an hour is performed, showing that the proposed laser can achieve stable mode-locking without the need for optical feedback or any other stabilization mechanism. (letter)

  8. 2 µm high-power dissipative soliton resonance in a compact σ-shaped Tm-doped double-clad fiber laser

    Science.gov (United States)

    Du, Tuanjie; Li, Weiwei; Ruan, Qiujun; Wang, Kaijie; Chen, Nan; Luo, Zhengqian

    2018-05-01

    We report direct generation of a high-power, large-energy dissipative soliton resonance (DSR) in a 2 µm Tm-doped double-clad fiber laser. A compact σ-shaped cavity is formed by a fiber Bragg grating and a 10/90 fiber loop mirror (FLM). The 10/90 FLM is not only used as an output mirror, but also acts as a nonlinear optical loop mirror for initiating mode locking. The mode-locked laser can deliver high-power, nanosecond DSR pulses at 2005.9 nm. We further perform a comparison study of the effect of the FLM’s loop length on the mode-locking threshold, peak power, pulse energy, and optical spectrum of the DSR pulses. We achieve a maximum average output power as high as 1.4 W, a maximum pulse energy of 353 nJ, and a maximum peak power of 84 W. This is, to the best of our knowledge, the highest power for 2 µm DSR pulses obtained in a mode-locked fiber laser.

  9. High-efficiency ytterbium-free erbium-doped all-glass double cladding silicate glass fiber for resonantly-pumped fiber lasers.

    Science.gov (United States)

    Qiang, Zexuan; Geng, Jihong; Luo, Tao; Zhang, Jun; Jiang, Shibin

    2014-02-01

    A highly efficient ytterbium-free erbium-doped silicate glass fiber has been developed for high-power fiber laser applications at an eye-safe wavelength near 1.55 μm. Our preliminary experiments show that high laser efficiency can be obtained from a relatively short length of the gain fiber when resonantly pumped at 1535 nm in both core- and cladding-pumping configurations. With a core-pumping configuration as high as 75%, optical-to-optical efficiency and 4 W output power were obtained at 1560 nm from a 1 m long gain fiber. When using a cladding-pumping configuration, approximately 13 W output power with 67.7% slope efficiency was demonstrated from a piece of 2 m long fiber. The lengths of silicate-based gain fiber are much shorter than their silica-based counterparts used in other experiments, which is significantly important for high-power narrow-band and/or pulsed laser applications.

  10. Resonant-bar gravitational radiation antennas

    International Nuclear Information System (INIS)

    Blair, D.G.

    1987-01-01

    This paper reviews the concept of gravitational radiation, and describes the worldwide research programme for the development of high-sensitivity resonant-bar antennas which are aimed at detecting gravitational radiation from astrophysical sources. (author)

  11. Investigations of elementary reactions of the methyl radical with the aid of laser magnetic resonance; Untersuchungen von Elementarreaktionen des Methylradikals mit Hilfe der Laser-Magnetischen-Resonanz

    Energy Technology Data Exchange (ETDEWEB)

    Deters, R.J.

    1998-01-01

    Selected elementary reactions of CH{sub 3} radicals in an isothermal flow system in the gaseous phase were investigated by means of LMR. [Deutsch] In dieser Arbeit wurden ausgewaehlte Elementarreaktionen von CH{sub 3}-Radikalen in einem isothermen Stroemungssystem in der Gasphase mit Hilfe der Laser-Magnetischen-Resonanz untersucht. (orig.)

  12. Demodulation method for tilted fiber Bragg grating refractometer with high sensitivity

    Science.gov (United States)

    Pham, Xuantung; Si, Jinhai; Chen, Tao; Wang, Ruize; Yan, Lihe; Cao, Houjun; Hou, Xun

    2018-05-01

    In this paper, we propose a demodulation method for refractive index (RI) sensing with tilted fiber Bragg gratings (TFBGs). It operates by monitoring the TFBG cladding mode resonance "cut-off wavelengths." The idea of a "cut-off wavelength" and its determination method are introduced. The RI sensitivities of TFBGs are significantly enhanced in certain RI ranges by using our demodulation method. The temperature-induced cross sensitivity is eliminated. We also demonstrate a parallel-double-angle TFBG (PDTFBG), in which two individual TFBGs are inscribed in the fiber core in parallel using a femtosecond laser and a phase mask. The RI sensing range of the PDTFBG is significantly broader than that of a conventional single-angle TFBG. In addition, its RI sensitivity can reach 1023.1 nm/refractive index unit in the 1.4401-1.4570 RI range when our proposed demodulation method is used.

  13. Intra-Cavity Total Reflection For High Sensitivity Measurement Of Optical Properties

    Science.gov (United States)

    Pipino, Andrew Charles Rule

    1999-11-16

    An optical cavity resonator device is provided for conducting sensitive murement of optical absorption by matter in any state with diffraction-limited spatial resolution through utilization of total internal reflection within a high-Q (high quality, low loss) optical cavity. Intracavity total reflection generates an evanescent wave that decays exponentially in space at a point external to the cavity, thereby providing a localized region where absorbing materials can be sensitively probed through alteration of the Q-factor of the otherwise isolated cavity. When a laser pulse is injected into the cavity and passes through the evanescent state, an amplitude loss resulting from absorption is incurred that reduces the lifetime of the pulse in the cavity. By monitoring the decay of the injected pulse, the absorption coefficient of manner within the evanescent wave region is accurately obtained from the decay time measurement.

  14. Resonant ionization by laser beams: application to ions sources and to study the nuclear structure of radioactive tellurium isotopes; Ionisation resonante par faisceaux laser: application aux sources d'ions et a l'etude de la structure des noyaux radioactifs de tellure

    Energy Technology Data Exchange (ETDEWEB)

    Sifi, R

    2007-07-15

    The radioactive ion beams that are produced through current isotope separators are well separated according to the A mass but not according to the Z parameter. The resonant ionization through laser beams applied to ion sources allows the production of radioactive ion beam in a very selective and efficient way by eliminating the isobaric contamination. The first chapter is dedicated to the resonant ionization by laser beams, we describe the principle, the experimental setting, the lasers used, the ionization schemes and the domain of application. The second chapter deals with the application of resonant ionization to laser ion sources for the production of radioactive ion beams. We present experimental tests performed for getting copper ion beams. Resonant ionization through laser is also used in the spectroscopy experiments performed at the Isolde (isotope separation on-line device) installation in CERN where more than 20 elements are ionized very efficiently. The technique is based on a frequency scanning around the excitation transition of the atoms in order to probe the hyperfine structure. Laser spectroscopy allows the determination of the hyperfine structure as well as the isotopic shift of atoms. In the third chapter the method is applied to the spectroscopy of tellurium atoms. First, we define the 2 parameters on which the extraction is based: charge radius and nuclear moments, then we present several theoretical models that we have used to assess our experimental results. (A.C.)

  15. Authentication Sensing System Using Resonance Evaluation Spectroscopy (ASSURES)

    Science.gov (United States)

    Trolinger, James D.; Dioumaev, Andrei K.; Lal, Amit K.; Dimas, Dave

    2017-08-01

    This paper describes an ongoing instrument development project to distinguish genuine manufactured components from counterfeit components; we call the instrument ASSURES (Authentication Sensing System Using Resonance Evaluation Spectroscopy). The system combines Laser Doppler Vibrometry with acoustical resonance spectroscopy, augmented with finite element analysis. Vibrational properties of components, such as resonant modes, damping, and spectral frequency response to various forcing functions depend strongly upon the mechanical properties of the material, including its size, shape, internal hardness, tensile strength, alloy/composite compositions, flaws, defects, and other internal material properties. Although acoustic resonant spectroscopy has seen limited application, the information rich signals in the vibrational spectra of objects provide a pathway to many new applications. Components with the same shape but made of different materials, different fatigue histories, damage, tampering, or heat treatment, will respond differently to high frequency stimulation. Laser Doppler Vibrometry offers high sensitivity and frequency bandwidth to measure the component's frequency spectrum, and overcomes many issues that limit conventional acoustical resonance spectroscopy, since the sensor laser beam can be aimed anywhere along the part as well as to multiple locations on a part in a non-contact way. ASSURES is especially promising for use in additive manufacturing technology by providing signatures as digital codes that are unique to specific objects and even to specific locations on objects. We believe that such signatures can be employed to address many important issues in the manufacturing industry. These include insuring the part meets the often very rigid specifications of the customer and being able to detect non-visible internal manufacturing defects or non-visible damage that has occurred after manufacturing.

  16. Plasma Levels of High Sensitivity Cardiac Troponin T in Adults with Repaired Tetralogy of Fallot

    Science.gov (United States)

    Lai, Clare T. M.; Wong, Sophia J.; Ip, Janice J. K.; Wong, Wai-keung; Tsang, Kwong-cheong; Lam, Wendy W. M.; Cheung, Yiu-fai

    2015-01-01

    Detectable low circulating level of cardiac troponin T (cTnT) may reflect subclinical myocardial injury. We tested the hypothesis that circulating levels of hs-cTnT are altered in adults with repaired tetralogy of Fallot (TOF) and associated with ventricular volume load and function. Eighty-eight TOF patients and 48 controls were studied. Plasma hs-cTnT levels were determined using a highly sensitive assay (hs-cTnT). The right (RV) and left ventricular (LV) volumes and ejection fraction (EF) were measured using 3D echocardiography and, in 52 patients, cardiac magnetic resonance (CMR). The median (interquartile range) for male and female patients were 4.87 (3.83–6.62) ng/L and 3.11 (1.00–3.87) ng/L, respectively. Thirty percent of female but none of the male patients had increased hs-cTnT levels. Female patients with elevated hs-cTnT levels, compared to those without, had greater RV end-diastolic and end-systolic volumes and LV systolic dyssynchrony index (all p < 0.05). For patient cohort only, hs-cTnT levels correlated positively with CMR-derived RV end-diastolic volume and negatively with echocardiography-derived LV and RV EF (all p < 0.05). Multiple linear regression identified sex and RV EF as significant correlates of log-transformed hs-cTnT levels. Increased hs-cTnT levels occur in 30% of female patients after TOF repair, and are associated with greater RV volumes and worse RV EF. PMID:26360613

  17. Highly sensitive detection of bovine serum albumin based on the aggregation of triangular silver nanoplates

    Science.gov (United States)

    Zhang, Ling Ling; Ma, Fang Fang; Kuang, Yang Fang; Cheng, Shu; Long, Yun Fei; Xiao, Qiu Guo

    2016-02-01

    A simple, fast and highly sensitive spectrophotometric method for the determination of bovine serum albumin (BSA) has been developed based on the interactions between triangular silver nanoplates (TAgNPs) and BSA in the presence of Britton-Robison buffer solution (BR). Particularly, the wavelength of absorption maximum (λmax) of TAgNPs is red shifted in the presence of BSA together with Britton-Robinson buffer solution (BR, pH = 2.56), and the color of the solution changed from blue to light blue. This may be due to the interactions between BSA molecules on the surface of TAgNPs through electrostatic forces, hydrogen bonds, hydrophobic effects and van der Waals forces at pH 2.56, which leads to the aggregation of TAgNPs. The determination of BSA was achieved by measuring the change of λmax corresponding to localized surface plasmon resonance (LSPR) from UV-visible spectrophotometry. It was found that the shift value in the wavelength of absorption maximum (Δλ, the difference in absorption maxima of the TAgNPs/BSA/BR mixture and the TAgNPs/BR mixture) was proportionate to the concentration of BSA in the range of 1.0 ng mL- 1 to 100.0 ng mL- 1 with the correlation coefficient of r = 0.9969. The detection limit (3 σ/k) for BSA was found to be as low as 0.5 ng mL- 1.

  18. A luminescent Lanthanide-free MOF nanohybrid for highly sensitive ratiometric temperature sensing in physiological range.

    Science.gov (United States)

    Zhou, You; Zhang, Denan; Zeng, Jin; Gan, Ning; Cuan, Jing

    2018-05-01

    Luminescent MOF materials with tunable emissions and energy/charge transfer processes have been extensively explored as ratiometric temperature sensors. However, most of the ratiometric MOF thermometers reported thus far are based on the MOFs containing photoactive lanthanides, which are potentially facing cost issue and serious supply shortage. Here, we present a ratiometric luminescent thermometer based on a dual-emitting lanthanide-free MOF hybrid, which is developed by encapsulation of a fluorescent dye into a robust nanocrystalline zirconium-based MOF through a one-pot synthesis approach. The structure and morphology of the hybrid product was characterized by Powder X-ray diffraction (PXRD), N 2 adsorption-desorption measurement and Scanning electron microscopy (SEM). The pore confinement effect well isolates the guest dye molecules and therefore suppresses the nonradiative energy transfer process between dye molecules. The incorporated dye emission is mainly sensitized by the organic linkers within MOF through fluorescence resonance energy transfer. The ratiometric luminescence of the MOF hybrid shows a significant response to temperature due to the thermal-related back energy transfer process from dye molecules and organic linkers, thus can be exploited for self-calibrated temperature sensing. The maximum thermometric sensitivity is 1.19% °C -1 in the physiological temperature range, which is among the highest for the ratiomtric MOF thermometers that operating in 25-45°C. The temperature resolution is better than 0.1°C over the entire operative range (20-60°C). By integrating the advantages of excellent stability, nanoscale nature, and high sensitivity and precision in the physiological temperature range, this dye@MOF hybrid might have potential application in biomedical diagnosis. What' more, this work has expanded the possibility of non-lanthanide luminescent MOF materials for the development of ratiometric temperature sensors. Copyright © 2018

  19. Fast and eco-friendly fabrication of uniform Ag substrates for highly sensitive surface-enhanced Raman scattering

    Science.gov (United States)

    Xu, Yongda; Li, Xin; Jiang, Lan; Meng, Ge; Ran, Peng; Lu, Yongfeng

    2017-05-01

    This study proposed a fast, simple, eco-friendly method for obtaining highly sensitive and uniform surface-enhanced Raman scattering (SERS) of silver (Ag) nanotextured substrates decorated with silver nanoparticles in open air. By splitting conventional femtosecond pulses (subpulse delay Δt = 0 ps) into pulse trains (subpulse delay Δt = 3 ps), the mean diameter of Ag nanoparticles was reduced by almost half and the amount of Ag nanoparticles with a diameter ranging from 20 to 60 nm was increased by more than 11 times. The substrate fabricated by femtosecond pulse trains has four main merits as follows: (1) High sensitivity: the maximum SERS enhancement factor is 1.26 × 109; (2) High efficiency: the fabrication rate can be up to 1600 μm2/s, which is 20-40 times faster than femtosecond photochemical reduction; (3) Good reproducibility: the relative standard deviation of the Raman signal intensity is 10.7%, which is one-third of that for conventional femtosecond laser; (4) Eco-friendly fabrication: neither chemical reagents nor vacuum conditions are needed during the fabrication process.

  20. Compact 1 mJ fiber MOPA for space-based laser-ablation resonant ionization mass spectrometry (LARIMS)

    Science.gov (United States)

    Mu, Xiaodong; Crain, William; Nguyen, Can; Ionov, Pavel; Steinvurzel, Paul; Dotan, Yaniv; Karuza, Petras; Lotshaw, William; Rose, Todd; Beck, Steven; Anderson, F. Scott

    2018-02-01

    A 1064 nm, 1 mJ pulsed fiber MOPA module, housed in 16"x14"x2.5" package for application in a lunar and planetary in-situ surface dating instrument is demonstrated. The module is based on a three-stage MOPA with a 60 μm core tapered fiber terminal amplifier. The master oscillator and first two preamplifier stages, which generate 20 μJ pulses, are all contained on a 13"x11"x1" board. Several improvements to the electronic signal control were instrumental to the laser development, including bipolar drive of the phase modulator for SBS suppression, shaping of the seed pulse to compensate pulse steepening, and pulsed operation of the power amplifier pump to reduce spontaneous emission at low pulse repetition frequency. The packaged laser runs at a repetition rate of 10 kHz and generates 10 ns pulses at 1 mJ with a 40 GHz linewidth, an M2 1.2 beam quality, and an 18 dB polarization extinction ratio. The modular design enables seven independent lasers to be stacked in a 20"x18"x16.25" enclosure, supporting a path towards a fiber laser based LARIMS for advanced materials characterization and chronological dating in harsh and remote environments.