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Sample records for high-energy spallation reactions

  1. High-energy nuclear reaction mechanisms - fission, fragmentation and spallation

    International Nuclear Information System (INIS)

    Kaufman, S.B.

    1987-01-01

    Measurements of the correlations in kinetic energy, mass, charge, and angle of coincident fragments formed in high-energy nuclear reactions have helped to characterize the processes of fission, fragmentation and spallation. For example, fission or fission-like two-body breakup mechanisms result in a strong angular correlation between two heavy fragments; in addition, the momentum transfer in the reaction can be deduced from the correlation. Another example is the multiplicity of light charged particles associated with a given heavy fragment, which is a measure of the violence of the collision, thus distinguishing between central and peripheral collisions. A summary of what has been learned about these processes from such studies will be given, along with some suggestions for further experiments

  2. Fragment mass distribution of proton-induced spallation reaction with intermediate energy

    International Nuclear Information System (INIS)

    Fan Sheng; Ye Yanlin; Xu Chuncheng; Chen Tao; Sobolevsky, N.M.

    2000-01-01

    The test of part benchmark of SHIELD code is finished. The fragment cross section and mass distribution and excitation function of the residual nuclei from proton-induced spallation reaction on thin Pb target with intermediate energy have been calculated by SHIELD code. And the results are in good agreement with measured data. The fragment mass distribution of the residual nuclei from proton-induced spallation reaction on thick Pb target with incident energy 1.6 GeV have been simulated

  3. Multi-criteria comparative evaluation of spallation reaction models

    Science.gov (United States)

    Andrianov, Andrey; Andrianova, Olga; Konobeev, Alexandr; Korovin, Yury; Kuptsov, Ilya

    2017-09-01

    This paper presents an approach to a comparative evaluation of the predictive ability of spallation reaction models based on widely used, well-proven multiple-criteria decision analysis methods (MAVT/MAUT, AHP, TOPSIS, PROMETHEE) and the results of such a comparison for 17 spallation reaction models in the presence of the interaction of high-energy protons with natPb.

  4. High energy nuclear reactions ('Spallation') and their application in calculation of the Acceleration Driven Systems (ADS)

    International Nuclear Information System (INIS)

    Rossi, Pedro Carlos Russo

    2011-01-01

    This work presents a study of high energy nuclear reactions which are fundamental to dene the source term in accelerator driven systems. These nuclear reactions, also known as spallation, consist in the interaction of high energetic hadrons with nucleons in the atomic nucleus. The phenomenology of these reactions consist in two step. In the rst, the proton interacts through multiple scattering in a process called intra-nuclear cascade. It is followed by a step in which the excited nucleus, coming from the intranuclear cascade, could either, evaporates particles to achieve a moderate energy state or fission. This process is known as competition between evaporation and fission. In this work the main nuclear models, Bertini and Cugnon are reviewed, since these models are fundamental for design purposes of the source term in ADS, due to lack of evaluated nuclear data for these reactions. The implementation and validation of the calculation methods for the design of the source is carried out to implement the methodology of source design using the program MCNPX (Monte Carlo N-Particle eXtended), devoted to calculation of transport of these particles and the validation performed by an international cooperation together with a Coordinated Research Project (CRP) of the International Atomic Energy Agency and available jobs, in order to qualify the calculations on nuclear reactions and the de-excitation channels involved, providing a state of the art of design and methodology for calculating external sources of spallation for source driven systems. The CRISP, is a brazilian code for the phenomenological description of the reactions involved and the models implemented in the code were reviewed and improved to continue the qualification process. Due to failure of the main models in describing the production of light nuclides, the multifragmentation reaction model was studied. Because the discrepancies in the calculations of production of these nuclides are attributes to the

  5. Spallation reactions: calculations

    International Nuclear Information System (INIS)

    Bertini, H.W.

    1975-01-01

    Current methods for calculating spallation reactions over various energy ranges are described and evaluated. Recent semiempirical fits to existing data will probably yield the most accurate predictions for these reactions in general. However, if the products in question have binding energies appreciably different from their isotropic neighbors and if the cross section is approximately 30 mb or larger, then the intranuclear-cascade-evaporation approach is probably better suited. (6 tables, 12 figures, 34 references) (U.S.)

  6. Mass formula dependence of calculated spallation reaction product distributions

    International Nuclear Information System (INIS)

    Nishida, Takahiko; Nakahara, Yasuaki

    1990-01-01

    A new version of the spallation reaction simulation code NUCLEUS was developed by incorporating Uno and Yamada's mass formula. This version was used to calculate the distribution of products from the spallation of uranium nuclei by high-energy protons. The dependence of the distributions on the mass formula was examined by comparing the results with those from the original version, which is based on Cameron's mass formula and the mass table compiled by Wapstra et al. As regards the fission component of spallation products, the new version reproduces the reaction product data obtained from thin foil experiments much better, especially on the neutron excess side. (orig.) [de

  7. Photonuclear spallation reactions in Cu

    International Nuclear Information System (INIS)

    Shibata, S.; Imamura, M.; Miyachi, T.

    1986-06-01

    Formation yields of 24 radioactive nuclides by the interaction of bremsstrahlung in the maximum end-point energies of 100 MeV - 1 GeV with Cu have been measured by direct γ-ray counting of irradiated targets. The yields in the mass range of 42 to 60 except for 60 Cu were analysed by non-linear least-squares fit to construct the mass yield and charge dispersion curves in spallation reactions. From the parameter values obtained, the energy dependence of the slope of the mass yield curve and the relationship between target N/Z and the most probable product N/Z were investigated in comparison with the results of proton, α and heavy ion-induced spallations of Cu. The characteristics of photon-induced spallations are discussed. (author)

  8. Energy dependence of isotopic spectra from spallation residues; Dependance en energie des spectres isotopiques de residus de spallation

    Energy Technology Data Exchange (ETDEWEB)

    Audouin, L

    2003-09-01

    Spallation reactions are collisions between heavy nuclei and light particle with an energy of a few hundreds MeV. The y are considered as a suitable way to create high- flux neutrons sources, which may used for example for the transmutation of nuclear wastes (hybrid reactors). The study of the residues from such reactions is both a way to understand the physics of the spallation and to provide information required for the design of industrial targets. The residues from the spallation of lead by proton at 500 MeV have been measured using the inverse kinematics technique in the FRS (fragments recoil separator). spectrometer from GSI (Barmstadt). This low energy required the use of new technique, for the experimental setup as well as during the analysis. The fragments were identified in-flight, prior to {beta} decay. Complete isotopic distributions are obtained with an accuracy ranging between 10 and 30%. Detailed information on the reaction kinematics are also obtained. Data are in excellent agreement with radio-chemical measurements, and bring new insights about the spallation process. The comparison with data measured on the same system with an incident energy of 1 GeV allows to discuss the influence of the projectile energy on the residues formation. It is concluded that the independence of the shape of the isobaric production cross sections regarding mass and energy of the projectile is preserved at low incident energies. The behaviour of Monte-Carlo codes is discussed with respect to those sets of data. The calculations show an improving agreement with decreasing energy, indicating that high-energy phenomena, for which some common assumptions become questionable, are the main reason for the observed discrepancies. (author)

  9. A sistematical study of spallation reaction

    International Nuclear Information System (INIS)

    Foshina, M.

    1982-01-01

    A four-parameter semi-empirical formulae is proposed to calculate photo-spallation cross sections. This formulae is deduced starting from a nuclear model considered as a particle mixture without differences among them and the spallation phenomenous is considered as sucessive nucleon emission ruled by determined probability law. The formulae parameters are obtained from photo-spallation yields experimentally determined and available in literature. A variation study of the values of different parameters with the mass number of the 'seed' nucleus and incident energy is made. A parallel study for the spallation reactions induced by protons of a sampling of 720 data is also presented. (L.C.) [pt

  10. Spallation reactions - physics and applications

    International Nuclear Information System (INIS)

    Kelic, A.; Ricciardi, M.; Schmidt, K-H.

    2009-01-01

    Spallation reactions have become an ideal tool for studying the equation of state and thermal instabilities of nuclear matter. In astrophysics, the interactions of cosmic rays with the interstellar medium have to be understood in detail for deducing their original composition and their production mechanisms. Renewed interest in spallation reactions with protons around 1 GeV came up recently with the developments of spallation neutron sources. The project of an accelerator-driven system (ADS) as a technological solution for incinerating the radioactive waste even intensified the efforts for better understanding the physics involved in the spallation process. Experiments on spallation reactions were performed for determining the production cross sections and properties of particles, fragments and heavy residues. Traditional experiments on heavy residues, performed in direct kinematics, were limited to the direct observation of long-lived radioactive nuclides and did not provide detailed information on the kinematics of the reaction. Therefore, an innovative experimental method has been developed, based on inverse kinematics, which allowed to identify all reaction residues in-flight, using the high resolution magnetic spectrometer FRS of GSL Darmstadt. It also gives direct access to the reaction kinematics. An experimental campaign has been carried out in a Europe-wide collaboration, investigating the spallation of several nuclei ranging from 56 Fe to 238 U Complementary experiments were performed with a full-acceptance detection system, yielding total fission cross sections. Recently, another detection system using the large acceptance ALADIN dipole and the LAND neutron detector was introduced to measure light particles in coincidence with the heavy residues. Another intense activity was dedicated to developing codes, which cover nuclear reactions occurring in an ADS. The first phase of the reaction is successfully described by a sequence of quasi-free nucleon

  11. Energy dependence of isotopic spectra from spallation residues

    International Nuclear Information System (INIS)

    Audouin, L.

    2003-09-01

    Spallation reactions are collisions between heavy nuclei and light particle with an energy of a few hundreds MeV. The y are considered as a suitable way to create high- flux neutrons sources, which may used for example for the transmutation of nuclear wastes (hybrid reactors). The study of the residues from such reactions is both a way to understand the physics of the spallation and to provide information required for the design of industrial targets. The residues from the spallation of lead by proton at 500 MeV have been measured using the inverse kinematics technique in the FRS (fragments recoil separator). spectrometer from GSI (Barmstadt). This low energy required the use of new technique, for the experimental setup as well as during the analysis. The fragments were identified in-flight, prior to β decay. Complete isotopic distributions are obtained with an accuracy ranging between 10 and 30%. Detailed information on the reaction kinematics are also obtained. Data are in excellent agreement with radio-chemical measurements, and bring new insights about the spallation process. The comparison with data measured on the same system with an incident energy of 1 GeV allows to discuss the influence of the projectile energy on the residues formation. It is concluded that the independence of the shape of the isobaric production cross sections regarding mass and energy of the projectile is preserved at low incident energies. The behaviour of Monte-Carlo codes is discussed with respect to those sets of data. The calculations show an improving agreement with decreasing energy, indicating that high-energy phenomena, for which some common assumptions become questionable, are the main reason for the observed discrepancies. (author)

  12. On the nucleon effective mass role to the high energy proton spallation reactions

    Energy Technology Data Exchange (ETDEWEB)

    Santos, B.M., E-mail: biank_ce@if.uff.br [Instituto de Física, Universidade Federal Fluminense, Av. Gal. Milton Tavares de Souza, 24210-346 Niterói, RJ (Brazil); Instituto Militar de Engenharia, Praça General Tibúrcio 80, 22290-270 Rio de Janeiro, RJ (Brazil); Pinheiro, A.R.C. [Centro Brasileiro de Pesquisas Físicas, Rua Dr. Xavier Sigaud 150, 22290-180 Rio de Janeiro, RJ (Brazil); Universidade Federal do Acre, BR 364 km 04, 69920-900 Rio Branco, AC (Brazil); Gonçalves, M. [Comissão Nacional de Energia Nuclear, Rua General Severiano 90, 22290-901 Rio de Janeiro, RJ (Brazil); Duarte, S.B. [Centro Brasileiro de Pesquisas Físicas, Rua Dr. Xavier Sigaud 150, 22290-180 Rio de Janeiro, RJ (Brazil); Cabral, R.G. [Instituto Militar de Engenharia, Praça General Tibúrcio 80, 22290-270 Rio de Janeiro, RJ (Brazil)

    2016-04-15

    We explore the effect of the nucleon effective mass to the dynamic evolution of the rapid phase of proton–nucleus spallation reactions. The analysis of the relaxation time for the non-equilibrium phase is studied by variations in the effective mass parameter. We determine the final excitation energy of the hot residual nucleus at the end of cascade phase and the de-excitation of the nuclear system is carried out considering the competition of particle evaporation and fission processes. It was shown that the excitation energy depends of the hot compound residual nucleus at the end of the rapid phase on the changing effective mass. The multiplicity of particles was also analyzed in cascade and evaporation phase of the reaction. The use of nucleon effective mass during cascade phase can be considered as an effect of the many-body nuclear interactions not included explicitly in a treatment to the nucleon–nucleon interaction inside the nucleus. This procedure represents a more realistic scenario to obtain the neutron multiplicity generated in this reaction, which is a benchmark for the calculation of the neutronic in the ADS reactors.

  13. Investigation of GeV proton-induced spallation reactions

    International Nuclear Information System (INIS)

    Hilscher, D.; Herbach, C.-M.; Jahnke, U.

    2003-01-01

    A reliable and precise modeling of GeV proton-induced spallation reactions is indispensable for the design of the spallation module and the target station of future accelerator driven hybrid reactors (ADS) or spallation neutron sources (ESS), in particular, to provide precise predictions for the neutron production, the radiation damage of materials (window), and the production of radioactivity ( 3 H, 7 Be etc.) in the target medium. Detailed experimental nuclear data are needed for sensitive validations and improvements of the models, whose predictive power is strongly dependent on the correct physical description of the three main stages of a spallation reaction: (i) the Intra-Nuclear-Cascade (INC) with the fast heating of the target nucleus, (ii) the de-excitation due to pre-equilibrium emission including the possibility of multi-fragmentation, and (iii) the statistical decay of thermally excited nuclei by evaporation of light particles and fission in the case of heavy nuclei. Key experimental data for this endeavour are absolute production cross sections and energy spectra for neutrons and light charged-particles (LCPs), emission of composite particles prior and post to the attainment of an equilibrated system, distribution of excitation energies deposited in the nuclei after the INC, and fission probabilities. The correlations of these quantities are particularly important to detect and identify possible deficiencies of the theoretical modeling of the various stages of a spallation reaction. Systematic measurements of such data are furthermore needed over large ranges of target nuclei and incident proton energies. Such data has been measured with the NESSI detector. An overview of new and previous results will be given. (authors)

  14. Spallation reactions; Reactions de spallation

    Energy Technology Data Exchange (ETDEWEB)

    Cugon, J.

    1996-12-31

    Spallation reactions dominate the interactions of hadrons with nuclei in the GeV range (from {approx} 0.1 to {approx} 10 GeV). They correspond to a sometimes important ejection of light particles leaving most of the time a residue of mass commensurate with the target mass. The main features of the experimental data are briefly reviewed. The most successful theoretical model, namely the intranuclear cascade + evaporation model, is presented. Its physical content, results and possible improvements are critically discussed. Alternative approaches are shortly reviewed. (author). 84 refs.

  15. A model for consecutive spallation and fragmentation reactions in inverse kinematics at relativistic energies

    International Nuclear Information System (INIS)

    Napolitani, P.; Tassan-Got, L.; Bernas, M.; Armbruster, P.

    2003-04-01

    Secondary reactions induced by relativistic beams in inverse kinematics in a thick target are relevant in several fields of experimental physics and technology, like secondary radioactive beams, production of exotic nuclei close to the proton drip line, and cross-section measurements for applications of spallation reactions for energy production and incineration of nuclear wastes. A general mathematical formulation is presented and successively applied as a tool to disentangle the primary reaction yields from the secondary production in the measurement of fission of a 238 U projectile impinging on a proton target at the energy of 1 A GeV. (orig.)

  16. Overcoming High Energy Backgrounds at Pulsed Spallation Sources

    CERN Document Server

    Cherkashyna, Nataliia; DiJulio, Douglas D.; Khaplanov, Anton; Pfeiffer, Dorothea; Scherzinger, Julius; Cooper-Jensen, Carsten P.; Fissum, Kevin G.; Ansell, Stuart; Iverson, Erik B.; Ehlers, Georg; Gallmeier, Franz X.; Panzner, Tobias; Rantsiou, Emmanouela; Kanaki, Kalliopi; Filges, Uwe; Kittelmann, Thomas; Extegarai, Maddi; Santoro, Valentina; Kirstein, Oliver; Bentley, Phillip M.

    2015-01-01

    Instrument backgrounds at neutron scattering facilities directly affect the quality and the efficiency of the scientific measurements that users perform. Part of the background at pulsed spallation neutron sources is caused by, and time-correlated with, the emission of high energy particles when the proton beam strikes the spallation target. This prompt pulse ultimately produces a signal, which can be highly problematic for a subset of instruments and measurements due to the time-correlated properties, and different to that from reactor sources. Measurements of this background have been made at both SNS (ORNL, Oak Ridge, TN, USA) and SINQ (PSI, Villigen, Switzerland). The background levels were generally found to be low compared to natural background. However, very low intensities of high-energy particles have been found to be detrimental to instrument performance in some conditions. Given that instrument performance is typically characterised by S/N, improvements in backgrounds can both improve instrument pe...

  17. Spallation reactions studied with 4-detector arrays

    Indian Academy of Sciences (India)

    Recently there has been a renewed interest in the study of spallation reactions in basic nuclear physics as well as in potential applications. Spallation reactions induced by light projectiles (protons, antiprotons, pions, etc.) in the GeV range allow the formation of hot nuclei which do not suffer the collective excitations ...

  18. Spallation reactions and energy deposition in heavy target materials comparison of measurements and MC-calculations

    International Nuclear Information System (INIS)

    Filges, D.; Enke, M.; Galin, J.

    2001-01-01

    A renascence of interest for energetic proton induced production of neutrons originates recently by the inception of new projects for target stations of intense spallation neutron sources (like the planned European Spallation Source ESS), accelerator-driven nuclear reactors, nuclear waste transmutation and also the application for radioactive beams. Here we verify the predictive power of transport codes currently on the market by confronting observables and quantities of interest with an exhaustive matrix of benchmark data essentially coming from two experiments being performed at the Cooler Synchrotron COSY at Juelich. Program packages like HERMES, LCS or MCNPX master the prevision of reaction cross sections, hadronic interaction lengths, averaged neutron multiplicities and neutron multiplicity distributions in thick and thin(!) targets for a wide spectrum of incident proton energies, geometrical shapes and materials of the target. While also the observables related to the energy deposition in thick targets are in a good agreement with the model predictions, the production cross section measurements however for light charged particles on thin targets point out that problems exist within these models. (author)

  19. Nucleon and composite-particle production in spallation reactions studied with the multi-purpose detector NESSI

    International Nuclear Information System (INIS)

    Herbach, C.M.; Hilscher, D.; Jahnke, U.; Tishchenko, V.G.; Galin, J.; Lott, B.; Letourneau, A.; Peghaire, A.; Filges, D.; Goldenbaum, F.; Nuenighoff, K.; Schaal, H.; Sterzenbach, G.; Wohlmuther, M.; Pienkowski, L.; Kostecke, D.; Schroeder, W.U.; Toke, J.

    2003-01-01

    NESSI, a 4π-detector for neutrons and charged particles, was used in studies of proton-induced spallation reactions at the COSY facility. Due to the high detection efficiency of NESSI for particles evaporated from excited nuclei, measured particle multiplicities provide event-by-event information on the nuclear excitation energy. Data obtained for proton-induced reactions on thin targets ranging from Al to U and proton energies from 0.8 to 2.5 GeV are compared with model predictions. (orig.)

  20. Light particle production in spallation reactions induced by protons of 0.8-2.5 GeV incident kinetic energy

    International Nuclear Information System (INIS)

    Herbach, Claus-Michael; Enke, Michael; Boehm, Andreas

    2002-01-01

    Absolute production cross sections have been measured simultaneously for neutrons and light charged particles in 0.8-2.5 GeV proton induced spallation reactions for a series of target nuclei from aluminum up to uranium. The high detection efficiency both for neutral and charged evaporative particles provides an event-wise access to the amount of projectile energy dissipated into nuclear excitation. Various intra nuclear cascade plus evaporation models have been confronted with the experimental data showing large discrepancies for hydrogen and helium production. (author)

  1. Gamma-ray emission cross section from proton-incident spallation reaction

    International Nuclear Information System (INIS)

    Iga, Kiminori; Ishibashi, Kenji; Shigyo, Nobuhiro

    1996-01-01

    Gamma-ray emission double differential cross sections from proton-incident spallation reaction have been measured at incident energies of 0.8, 1.5 and 3.0 GeV with Al, Fe, In and Pb targets. The experimental results have been compared with calculate values of HETC-KFA2. The measured cross sections disagree with the calculated results in the gamma ray energies above 10 MeV. (author)

  2. Physics and technology of spallation neutron sources

    International Nuclear Information System (INIS)

    Bauer, G.S.

    1998-08-01

    Next to fission and fusion, spallation is an efficient process for releasing neutrons from nuclei. Unlike the other two reactions, it is an endothermal process and can, therefore, not be used per se in energy generation. In order to sustain a spallation reaction, an energetic beam of particles, most commonly protons, must be supplied onto a heavy target. Spallation can, however, play an important role as a source of neutrons whose flux can be easily controlled via the driving beam. Up to a few GeV of energy, the neutron production is roughly proportional to the beam power. Although sophisticated Monte Carlo codes exist to compute all aspects of a spallation facility, many features can be understood on the basis of simple physics arguments. Technically a spallation facility is very demanding, not only because a reliable and economic accelerator of high power is needed to drive the reaction, but also, and in particular, because high levels of radiation and heat are generated in the target which are difficult to cope with. Radiation effects in a spallation environment are different from those commonly encountered in a reactor and are probably even more temperature dependent than the latter because of the high gas production rate. A commonly favored solution is the use of molten heavy metal targets. While radiation damage is not a problem in this case, except for the container, a number of other issues are discussed. (author)

  3. Optimization of $^{178m2}$/Hf isomer production in spallation reactions at projectile energies up to 100 MeV using STAPRE and ALICE code simulations

    CERN Document Server

    Kirischuk, V I; Khomenkov, V P; Strilchuk, N V; Zheltonozhskij, V A

    2004-01-01

    /sup 178m2/Hf isomer production in different spallation reactions with protons, alpha particles and neutrons at projectile energies up to 100 MeV has been analyzed using both STAPRE and ALICE code simulations. The STAPRE code was used to calculate the isomeric ratios, while the ALICE code was used to simulate the excitation functions of the respective ground states. A number of spallation reactions have been compared taking into account not only /sup 178m2 /Hf isomer productivity but also, first, the isomeric ratios calculated by the STAPRE code; second, the accumulation of the most undesirable Hf isotopes and isomers, such as /sup 172/Hf, /sup 175 /Hf, and /sup 179m/Hf; and, third, the production of other admixtures and by-products that could degrade the quality of the produced /sup 178m2/Hf isomer sources, including all stable Hf isotopes as well. Possibilities and ways of optimizing /sup 178m2/Hf isomer production in spallation reactions at projectile energies up to 100 MeV are discussed. This can be consi...

  4. Cross-sections of spallation residues produced in Proton –Induced reactions

    International Nuclear Information System (INIS)

    Al-Haydari, A.; Khan, A.A.; Abdul Ganai, A.; Hassan, G.S.

    2013-01-01

    The recent available GSI data for proton-induced spallation reactions by using inverse kinematics at different energies are analyzed for different reactions in terms of the percolation model together with the intranuclear cascade model (MCAS). The simulation results obtained for the cross sections of production of light ions and isotopes as a function of mass and charge number is calculated. Results of calculations are in good agreement with experiment

  5. Results from the IAEA benchmark of spallation models

    International Nuclear Information System (INIS)

    Leray, S.; David, J.C.; Khandaker, M.; Mank, G.; Mengoni, A.; Otsuka, N.; Filges, D.; Gallmeier, F.; Konobeyev, A.; Michel, R.

    2011-01-01

    Spallation reactions play an important role in a wide domain of applications. In the simulation codes used in this field, the nuclear interaction cross-sections and characteristics are computed by spallation models. The International Atomic Energy Agency (IAEA) has recently organised a benchmark of the spallation models used or that could be used in the future into high-energy transport codes. The objectives were, first, to assess the prediction capabilities of the different spallation models for the different mass and energy regions and the different exit channels and, second, to understand the reason for the success or deficiency of the models. Results of the benchmark concerning both the analysis of the prediction capabilities of the models and the first conclusions on the physics of spallation models are presented. (authors)

  6. Spallation: understanding for predicting !?

    International Nuclear Information System (INIS)

    David, J.-C.

    2012-01-01

    This HDR report summarizes about ten years spent around spallation reaction modelling. Spallation reactions are defined as interaction of a light particle, say a nucleon, and a nucleus at an incident energy from 100 MeV up to 2-3 GeV. These reactions are divided in two steps. A first and fast phase, direct reactions also called intranuclear cascade, following by a slower phase, deexcitation of the remnant nucleus. Using the combination of INCL4, the intranuclear cascade model developed by the group, and the deexcitation code Abla from GSI, as a connecting thread, the multi-faceted spallation is presented. Chapter one deals with physics and codes, then different types of benchmarks are addressed, followed by several domains where spallation modelling plays a role, and finally, taking advantage of what has been said previously and of what can be read in the literature, new developments are suggested. (author) [fr

  7. Current status of high energy nucleon-meson transport code

    Energy Technology Data Exchange (ETDEWEB)

    Takada, Hiroshi; Sasa, Toshinobu [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

    1998-03-01

    Current status of design code of accelerator (NMTC/JAERI code), outline of physical model and evaluation of accuracy of code were reported. To evaluate the nuclear performance of accelerator and strong spallation neutron origin, the nuclear reaction between high energy proton and target nuclide and behaviors of various produced particles are necessary. The nuclear design of spallation neutron system used a calculation code system connected the high energy nucleon{center_dot}meson transport code and the neutron{center_dot}photon transport code. NMTC/JAERI is described by the particle evaporation process under consideration of competition reaction of intranuclear cascade and fission process. Particle transport calculation was carried out for proton, neutron, {pi}- and {mu}-meson. To verify and improve accuracy of high energy nucleon-meson transport code, data of spallation and spallation neutron fragment by the integral experiment were collected. (S.Y.)

  8. Shielding concerns at a spallation source

    International Nuclear Information System (INIS)

    Russell, G.J.; Robinson, H.; Legate, G.L.; Woods, R.

    1989-01-01

    Neutrons produced by 800-MeV proton reactions at the Los Alamos Neutron Scattering Center spallation neutron source cause a variety of challenging shielding problems. We identify several characteristics distinctly different from reactor shielding and compute the dose attenuation through an infinite slab/shield composed of iron (100 cm) and borated polyethylene (15 cm). Our calculations show that (for an incident spallation spectrum characteristic of neutrons leaking from a tungsten target at 90/degree/) the dose through the shield is a complex mixture of neutrons and gamma rays. High-energy (> 20 MeV) neutron production from the target is ≅5% of the total, yet causes ≅68% of the dose at the shield surface. Primary low-energy (< 20 MeV) neutrons from the target contribute negligibly (≅0.5%) to the dose at the shield surface yet cause gamma rays, which contribute ≅31% to the total dose at the shield surface. Low-energy neutrons from spallation reactions behave similarly to neutrons with a fission spectrum distribution. 6 refs., 8 figs., 1 tab

  9. Radiation physics of high power spallation targets. State of the art simulation methods and experiments, the 'European Spallation Source' (ESS)

    International Nuclear Information System (INIS)

    Filges, D.; Cloth, P.; Neef, R.D.; Schaal, H.

    1998-01-01

    Particle transport and nuclear interactions of planned high power spallation targets with GeV proton beams can be simulated using widely developed Monte Carlo transport methods. This includes available high energy radiation transport codes and systems for low energy, earlier developed for reactor physics and fusion technology. Monte Carlo simulation codes and applied methods are discussed. The capabilities of the world-wide existing state-of-the-art computer code systems are demonstrated. Results of computational studies for the 'European Spallation Source' (ESS) mercury high power target station are given. The needs for spallation related data and planned experiments are shown. (author)

  10. Status of spallation neutron source program in High Intensity Proton Accelerator Project

    International Nuclear Information System (INIS)

    Oyama, Yukio

    2001-01-01

    Japan Atomic Energy Research Institute and High Energy Accelerator Organization are jointly designing a 1 MW spallation neutron source as one of the research facilities planned in the High Intensity Proton Accelerator Project. The spallation neutron source is driven by 3 GeV proton beam with a mercury target and liquid hydrogen moderators. The present status of design for these spallation source and relevant facility is overviewed. (author)

  11. NMTC/JAM, Simulates High Energy Nuclear Reactions and Nuclear-Meson Transport Processes

    International Nuclear Information System (INIS)

    Furihata, Shiori

    2002-01-01

    1 - Description of program or function: NMTC/JAM is an upgraded version of the code system NMTC/JAERI97. NMTC/JAERI97 simulates high energy nuclear reactions and nucleon-meson transport processes. It implements an intra-nuclear cascade model taking account of the in-medium nuclear effects and the pre-equilibrium calculation model based on the exciton one. For treating the nucleon transport process, the nucleon-nucleus cross sections are revised to those derived by the systematics of Pearlstein. Moreover, the level density parameter derived by Ignatyuk is included as a new option for particle evaporation calculation. A geometry package based on the Combinatorial Geometry with multi-array system and the importance sampling technique is implemented in the code. Tally function is also employed for obtaining such physical quantities as neutron energy spectra, heat deposition and nuclide yield without editing a history file. The code can simulate both the primary spallation reaction and the secondary particle transport in the intermediate energy region from 20 MeV to 3.5 GeV by the use of the Monte Carlo technique. The code has been employed in combination with the neutron-photon transport codes available to the energy region below 20 MeV for neutronics calculation of accelerator-based subcritical reactors, analyses of thick target spallation experimented and so on. 2 - Methods: High energy nuclear reactions induced by incident high energy protons, neutrons and pions are simulated with the Monte Carlo Method by the intra-nuclear nucleon-nucleon reaction probabilities based on an intra-nuclear nucleon cascade model followed by the particle evaporation including high energy fission process. Jet-Aa Microscopic transport model (JAM) is employed to simulate high energy nuclear reactions in the energy range of GeV. All reaction channels are taken into account in the JAM calculation. An intra-nuclear cascade model (ISOBAR code) taking account of the in-medium nuclear effects

  12. EXPERIMENTAL ANALYSES OF SPALLATION NEUTRONS GENERATED BY 100 MEV PROTONS AT THE KYOTO UNIVERSITY CRITICAL ASSEMBLY

    Directory of Open Access Journals (Sweden)

    CHEOL HO PYEON

    2013-02-01

    Full Text Available Neutron spectrum analyses of spallation neutrons are conducted in the accelerator-driven system (ADS facility at the Kyoto University Critical Assembly (KUCA. High-energy protons (100 MeV obtained from the fixed field alternating gradient accelerator are injected onto a tungsten target, whereby the spallation neutrons are generated. For neutronic characteristics of spallation neutrons, the reaction rates and the continuous energy distribution of spallation neutrons are measured by the foil activation method and by an organic liquid scintillator, respectively. Numerical calculations are executed by MCNPX with JENDL/HE-2007 and ENDF/B-VI libraries to evaluate the reaction rates of activation foils (bismuth and indium set at the target and the continuous energy distribution of spallation neutrons set in front of the target. For the reaction rates by the foil activation method, the C/E values between the experiments and the calculations are found around a relative difference of 10%, except for some reactions. For continuous energy distribution by the organic liquid scintillator, the spallation neutrons are observed up to 45 MeV. From these results, the neutron spectrum information on the spallation neutrons generated at the target are attained successfully in injecting 100 MeV protons onto the tungsten target.

  13. Accelerator driven reactors, - the significance of the energy distribution of spallation neutrons on the neutron statistics

    Energy Technology Data Exchange (ETDEWEB)

    Fhager, V

    2000-01-01

    In order to make correct predictions of the second moment of statistical nuclear variables, such as the number of fissions and the number of thermalized neutrons, the dependence of the energy distribution of the source particles on their number should be considered. It has been pointed out recently that neglecting this number dependence in accelerator driven systems might result in bad estimates of the second moment, and this paper contains qualitative and quantitative estimates of the size of these efforts. We walk towards the requested results in two steps. First, models of the number dependent energy distributions of the neutrons that are ejected in the spallation reactions are constructed, both by simple assumptions and by extracting energy distributions of spallation neutrons from a high-energy particle transport code. Then, the second moment of nuclear variables in a sub-critical reactor, into which spallation neutrons are injected, is calculated. The results from second moment calculations using number dependent energy distributions for the source neutrons are compared to those where only the average energy distribution is used. Two physical models are employed to simulate the neutron transport in the reactor. One is analytical, treating only slowing down of neutrons by elastic scattering in the core material. For this model, equations are written down and solved for the second moment of thermalized neutrons that include the distribution of energy of the spallation neutrons. The other model utilizes Monte Carlo methods for tracking the source neutrons as they travel inside the reactor material. Fast and thermal fission reactions are considered, as well as neutron capture and elastic scattering, and the second moment of the number of fissions, the number of neutrons that leaked out of the system, etc. are calculated. Both models use a cylindrical core with a homogenous mixture of core material. Our results indicate that the number dependence of the energy

  14. Accelerator driven reactors, - the significance of the energy distribution of spallation neutrons on the neutron statistics

    International Nuclear Information System (INIS)

    Fhager, V.

    2000-01-01

    In order to make correct predictions of the second moment of statistical nuclear variables, such as the number of fissions and the number of thermalized neutrons, the dependence of the energy distribution of the source particles on their number should be considered. It has been pointed out recently that neglecting this number dependence in accelerator driven systems might result in bad estimates of the second moment, and this paper contains qualitative and quantitative estimates of the size of these efforts. We walk towards the requested results in two steps. First, models of the number dependent energy distributions of the neutrons that are ejected in the spallation reactions are constructed, both by simple assumptions and by extracting energy distributions of spallation neutrons from a high-energy particle transport code. Then, the second moment of nuclear variables in a sub-critical reactor, into which spallation neutrons are injected, is calculated. The results from second moment calculations using number dependent energy distributions for the source neutrons are compared to those where only the average energy distribution is used. Two physical models are employed to simulate the neutron transport in the reactor. One is analytical, treating only slowing down of neutrons by elastic scattering in the core material. For this model, equations are written down and solved for the second moment of thermalized neutrons that include the distribution of energy of the spallation neutrons. The other model utilizes Monte Carlo methods for tracking the source neutrons as they travel inside the reactor material. Fast and thermal fission reactions are considered, as well as neutron capture and elastic scattering, and the second moment of the number of fissions, the number of neutrons that leaked out of the system, etc. are calculated. Both models use a cylindrical core with a homogenous mixture of core material. Our results indicate that the number dependence of the energy

  15. High-energy neutrino background: Limitations on models of deuterium production

    International Nuclear Information System (INIS)

    Eichler, D.

    1979-01-01

    It is pointed out that Epstein's model for deuterium production via high-energy spallation reactions produces high-energy neutrinos in sufficient quantity to stand out above those that are produced by cosmic-ray interactions in the Earth's atmosphere. That the Reines experiment detected neutrinos of atmospheric origin without detecting any cosmic component restricts deuterium production by spallation reactions to very high redshifts (z> or approx. =300). Improved neutrino experiments may be able to push these limits back to recombination

  16. Development of a nuclear spallation simulation code and calculations of primary spallation products

    International Nuclear Information System (INIS)

    Nishida, Takahiko; Nakahara, Yasuaki; Tsutsui, Tsuneo

    1986-08-01

    In order to make evaluations of computational models for the nuclear spallation reaction from a nuclear physics point of view, a simulation code NUCLEUS has been developed by modifying and combining the Monte Carlo codes NMTC/JAERI and NMTA/JAERI for calculating only the nuclear spallation reaction (intranuclear cascade + evaporation and/or fast fission) between a nucleus and a projectile without taking into consideration of internuclear transport. New several plotting routines have been provided for the rapid process of much more event data, obtained by using the ARGUS plotting system. The results obtained by our code can be directly compared with the experimental results using by thin foil experiments in which internuclear multiple collisions have little effects, and will serve to upgrade the calculational methods and the values of nuclear parameters currently used in the calculations. Some discussions are done about the preliminary computational results obtained by using NUCLEUS. The mass distribution and charge dispersion of reaction products are examined in some detail for the nuclear spallation reaction between incident protons and target nuclei, such as U, Pb and Ag, in the energy range from 0.5 GeV to 3.0 GeV. These results show that the distribution of reaction products ceases to change its form as the proton energy increases over about 2 GeV. The same tendency is seen in the energy dependence of the number of primary particles emitted from a nucleus. After spallation reactions, a variety of nuclei, especially many neutron deficient nuclides with nuclear charges nearly equal to ones of a target nucleus, are produced. Due to their short lifetime most of them will change to stable nuclides in due time. Finally, some important issues are discussed to improve the present simulation method. (author)

  17. Validation of MC models of spallation reactions in thin and thick targets in the GeV range

    International Nuclear Information System (INIS)

    Goldenbaum, F.; Filges, D.; Neef, R.D.; Nuenighoff, K.; Paul, N.; Schaal, H.; Sterzenbach, G.; Tietze, A.; Wohlmuther, M.; Galin, J.; Letourneau, A.; Lott, B.; Peghaire, A.; Pienkowski, L.

    2001-01-01

    In the framework of new projects of intense spallation neutron sources an extensive experimental and theoretical effort is devoted to the precise prediction and optimization of the targets and shielding in terms of reaction cross sections, hadronic interaction lengths and usable neutrons produced in proton induced spallation reactions. Strong constraints on Monte-Carlo high energy transport codes are put by a measurement campaign of the NESSI (neutron scintillator and silicon detector) collaboration. While the predictive power of inter- and intra-nuclear cascade models coupled to evaporation codes and transport systems is excellent as far as neutron production in thick targets is concerned, there are considerable discrepancies not only between experiments and models, but also among the different codes themselves when regarding charged particle production in thin targets. In the current contribution a representative validation will be executed and possible deficiencies within the codes are elaborated. (orig.)

  18. Constraining statistical-model parameters using fusion and spallation reactions

    Directory of Open Access Journals (Sweden)

    Charity Robert J.

    2011-10-01

    Full Text Available The de-excitation of compound nuclei has been successfully described for several decades by means of statistical models. However, such models involve a large number of free parameters and ingredients that are often underconstrained by experimental data. We show how the degeneracy of the model ingredients can be partially lifted by studying different entrance channels for de-excitation, which populate different regions of the parameter space of the compound nucleus. Fusion reactions, in particular, play an important role in this strategy because they fix three out of four of the compound-nucleus parameters (mass, charge and total excitation energy. The present work focuses on fission and intermediate-mass-fragment emission cross sections. We prove how equivalent parameter sets for fusion-fission reactions can be resolved using another entrance channel, namely spallation reactions. Intermediate-mass-fragment emission can be constrained in a similar way. An interpretation of the best-fit IMF barriers in terms of the Wigner energies of the nascent fragments is discussed.

  19. Production of Actinium-225 via High Energy Proton Induced Spallation of Thorium-232

    Energy Technology Data Exchange (ETDEWEB)

    Harvey, James T.; Nolen, Jerry; Vandergrift, George; Gomes, Itacil; Kroc, Tom; Horwitz, Phil; McAlister, Dan; Bowers, Del; Sullivan, Vivian; Greene, John

    2011-12-30

    The science of cancer research is currently expanding its use of alpha particle emitting radioisotopes. Coupled with the discovery and proliferation of molecular species that seek out and attach to tumors, new therapy and diagnostics are being developed to enhance the treatment of cancer and other diseases. This latest technology is commonly referred to as Alpha Immunotherapy (AIT). Actinium-225/Bismuth-213 is a parent/daughter alpha-emitting radioisotope pair that is highly sought after because of the potential for treating numerous diseases and its ability to be chemically compatible with many known and widely used carrier molecules (such as monoclonal antibodies and proteins/peptides). Unfortunately, the worldwide supply of actinium-225 is limited to about 1,000mCi annually and most of that is currently spoken for, thus limiting the ability of this radioisotope pair to enter into research and subsequently clinical trials. The route proposed herein utilizes high energy protons to produce actinium-225 via spallation of a thorium-232 target. As part of previous R and D efforts carried out at Argonne National Laboratory recently in support of the proposed US FRIB facility, it was shown that a very effective production mechanism for actinium-225 is spallation of thorium-232 by high energy proton beams. The base-line simulation for the production rate of actinium-225 by this reaction mechanism is 8E12 atoms per second at 200 MeV proton beam energy with 50 g/cm2 thorium target and 100 kW beam power. An irradiation of one actinium-225 half-life (10 days) produces {approx}100 Ci of actinium-225. For a given beam current the reaction cross section increases slightly with energy to about 400 MeV and then decreases slightly for beam energies in the several GeV regime. The object of this effort is to refine the simulations at proton beam energies of 400 MeV and above up to about 8 GeV. Once completed, the simulations will be experimentally verified using 400 MeV and 8 Ge

  20. Status of helium-production reaction studies with a spallation neutron source

    International Nuclear Information System (INIS)

    Haight, R.C.; Bateman, F.B.; Chadwick, M.B.

    1994-01-01

    Alpha--particle production cross sections and spectra are being measured at the spallation source of fast neutrons at the Los Alamos Meson Physics Facility (LAMPF). Detectors at angles of 30, 60, 90 and 135 degree are used to identify alpha particles, measure their energy spectra, and indicate the time-of-flight, and hence the energy, of the neutrons inducing the reaction. The useful neutron energy ranges from less than 1 MeV to approximately 50 MeV for the present experimental setup. Targets under study at present include C, N, O, 27 Al, Si, 51 V, 56 Fe, 59 Co, 58,60 Ni, 89 Y and 93 Nb. Results for 59 Co illustrate the capabilities of the approach

  1. Spallation reactions in shock waves at supernova explosions and related problems

    Energy Technology Data Exchange (ETDEWEB)

    Ustinova, G. K., E-mail: ustinova@dubna.net.ru [RAS, V.I. Vernadsky Institute of Geochemistry and Analytical Chemistry (Russian Federation)

    2013-05-15

    The isotopic anomalies of some extinct radionuclides testify to the outburst of a nearby supernova just before the collapse of the protosolar nebula, and to the fact that the supernova was Sn Ia, i.e. the carbon-detonation supernova. A key role of spallation reactions in the formation of isotopic anomalies in the primordial matter of the Solar System is revealed. It is conditioned by the diffusive acceleration of particles in the explosive shock waves, which leads to the amplification of rigidity of the energy spectrum of particles and its enrichment with heavier ions. The quantitative calculations of such isotopic anomalies of many elements are presented. It is well-grounded that the anomalous Xe-HL in meteoritic nanodiamonds was formed simultaneously with nanodiamonds themselves during the shock wave propagation at the Sn Ia explosion. The possible effects of shock wave fractionation of noble gases in the atmosphere of planets are considered. The origin of light elements Li, Be and B in spallation reactions, predicted by Fowler in the middle of the last century, is argued. All the investigated isotopic anomalies give the evidence for the extremely high magnetohydrodynamics (MHD) conditions at the initial stage of free expansion of the explosive shock wave from Sn Ia, which can be essential in solution of the problem of origin of cosmic rays. The specific iron-enriched matter of Sn Ia and its MHD-separation in turbulent processes must be taking into account in the models of origin of the Solar System.

  2. Introduction to spallation physics and spallation-target design

    Energy Technology Data Exchange (ETDEWEB)

    Russell, G.J.; Pitcher, E.J.; Daemen, L.L. [Los Alamos National Laboratory, NM (United States)

    1995-10-01

    When coupled with the spallation process in appropriate target materials, high-power accelerators can be used to produce large numbers of neutrons, thus providing an alternate method to the use of nuclear reactors for this purpose. Spallation offers exciting new possibilities for generating intense neutron fluxes for a variety of applications, including: (a) spallation-neutron sources for materials science research; (b) accelerator-based production of tritium; (c) accelerator-based transmutation of waste; (d) accelerator-based destruction of plutonium; and (e) radioisotope production for medical and energy applications. Target design plays a key role in these applications, with neutron production/leakage being strongly dependent on the incident particle type and energy, and target material and geometry.

  3. Analysis for mass distribution of proton-induced reactions in intermediate energy range

    CERN Document Server

    Xiao Yu Heng

    2002-01-01

    The mass and charge distribution of residual products produced in the spallation reactions needs to be studied, because it can provide useful information for the disposal of nuclear waste and residual radioactivity generated by the spallation neutron target system. In present work, the Many State Dynamical Model (MSDM) is based on the Cascade-Exciton Model (CEM). The authors use it to investigate the mass distribution of Nb, Au and Pb proton-induced reactions in energy range from 100 MeV to 3 GeV. The agreement between the MSDM simulations and the measured data is good in this energy range, and deviations mainly show up in the mass range of 90 - 150 for the high energy proton incident upon Au and Pb

  4. Dissertation: Precompound Emission of Energetic Light Fragments in Spallation Reactions

    Energy Technology Data Exchange (ETDEWEB)

    Kerby, Leslie Marie [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

    2015-08-04

    Emission of light fragments (LF) from nuclear reactions is an open question. Different reaction mechanisms contribute to their production; the relative roles of each, and how they change with incident energy, mass number of the target, and the type and emission energy of the fragments is not completely understood. None of the available models are able to accurately predict emission of LF from arbitrary reactions. However, the ability to describe production of LF (especially at energies ≳ 30 MeV) from many reactions is important for different applications, such as cosmic-ray-induced Single Event Upsets (SEUs), radiation protection, and cancer therapy with proton and heavy-ion beams, to name just a few. The Cascade-Exciton Model (CEM) version 03.03 and the Los Alamos version of the Quark-Gluon String Model (LAQGSM) version 03.03 event generators in Monte Carlo N-Particle Transport Code version 6 (MCNP6) describe quite well the spectra of fragments with sizes up to ⁴He across a broad range of target masses and incident energies (up to ~ 5 GeV for CEM and up to ~ 1 TeV/A for LAQGSM). However, they do not predict the high energy tails of LF spectra heavier than ⁴He well. Most LF with energies above several tens of MeV are emitted during the precompound stage of a reaction. The current versions of the CEM and LAQGSM event generators do not account for precompound emission of LF larger than ⁴He. The aim of our work is to extend the precompound model in them to include such processes, leading to an increase of predictive power of LF-production in MCNP6. This entails upgrading the Modified Exciton Model currently used at the preequilibrium stage in CEM and LAQGSM. It also includes expansion and examination of the coalescence and Fermi break-up models used in the precompound stages of spallation reactions within CEM and LAQGSM. Extending our models to include emission of fragments heavier than ⁴He at the precompound stage has indeed provided results that have much

  5. Modelling of the spallation reaction: analysis and testing of nuclear models

    International Nuclear Information System (INIS)

    Toccoli, C.

    2000-01-01

    The spallation reaction is considered as a 2-step process. First a very quick stage (10 -22 , 10 -29 s) which corresponds to the individual interaction between the incident projectile and nucleons, this interaction is followed by a series of nucleon-nucleon collisions (intranuclear cascade) during which fast particles are emitted, the nucleus is left in a strongly excited level. Secondly a slower stage (10 -18 , 10 -19 s) during which the nucleus is expected to de-excite completely. This de-excitation is performed by evaporation of light particles (n, p, d, t, 3 He, 4 He) or/and fission or/and fragmentation. The HETC code has been designed to simulate spallation reactions, this simulation is based on the 2-steps process and on several models of intranuclear cascades (Bertini model, Cugnon model, Helder Duarte model), the evaporation model relies on the statistical theory of Weiskopf-Ewing. The purpose of this work is to evaluate the ability of the HETC code to predict experimental results. A methodology about the comparison of relevant experimental data with results of calculation is presented and a preliminary estimation of the systematic error of the HETC code is proposed. The main problem of cascade models originates in the difficulty of simulating inelastic nucleon-nucleon collisions, the emission of pions is over-estimated and corresponding differential spectra are badly reproduced. The inaccuracy of cascade models has a great impact to determine the excited level of the nucleus at the end of the first step and indirectly on the distribution of final residual nuclei. The test of the evaporation model has shown that the emission of high energy light particles is under-estimated. (A.C.)

  6. On the role of secondary pions in spallation targets

    Energy Technology Data Exchange (ETDEWEB)

    Mancusi, Davide [Paris-Saclay Univ., Gif-sur-Yvette (France). Den-Service d' Etude des Reacteurs et de Mathematiques Appliquees (SERMA); Lo Meo, Sergio [ENEA, Research Centre ' ' Ezio Clementel' ' , Bologna (Italy); INFN, Bologna (Italy); Colonna, Nicola [INFN, Bari (Italy); Boudard, Alain; David, Jean-Christophe; Leray, Sylvie [Paris-Saclay Univ., Gif-sur-Yvette (France). IRFU, CEA; Cortes-Giraldo, Miguel Antonio; Lerendegui-Marco, Jorge [Sevilla Univ. (Spain). Facultad de Fisica; Cugnon, Joseph [Liege Univ. (Belgium). AGO Dept.; Massimi, Cristian [INFN, Bologna (Italy); Bologna Univ. (Italy). Physics and Astronomy Dept.; Vlachoudis, Vasilis [European Organization for Nuclear Research (CERN), Geneva (Switzerland)

    2017-05-15

    We use particle-transport simulations to show that secondary pions play a crucial role for the development of the hadronic cascade and therefore for the production of neutrons and photons from thick spallation targets. In particular, for the nTOF lead spallation target, irradiated with 20 GeV/c protons, neutral pions are involved in the production of ∝ 90% of the high-energy photons; charged pions participate in ∝ 40% of the integral neutron yield. Nevertheless, photon and neutron yields are shown to be relatively insensitive to large changes of the average pion multiplicity in the individual spallation reactions. We characterize this robustness as a peculiar property of hadronic cascades in thick targets. (orig.)

  7. On the role of secondary pions in spallation targets

    CERN Document Server

    Mancusi, Davide; Colonna, Nicola; Boudard, Alain; Cortés-Giraldo, Miguel Antonio; Cugnon, Joseph; David, Jean-Christophe; Leray, Sylvie; Lerendegui-Marco, Jorge; Massimi, Cristian; Vlachoudis, Vasilis

    2017-01-01

    We use particle-transport simulations to show that secondary pions play a crucial role for the development of the hadronic cascade and therefore for the production of neutrons and photons from thick spallation targets. In particular, for the n_TOF lead spallation target, irradiated with 20-GeV/c protons, neutral pions are involved in the production of ~90% of the high-energy photons; charged pions participate in ~40% of the integral neutron yield. Nevertheless, photon and neutron yields are shown to be relatively insensitive to large changes of the average pion multiplicity in the individual spallation reactions. We characterize this robustness as a peculiar property of hadronic cascades in thick targets.

  8. Helium production for 0.8-2.5 GeV proton induced spallation reactions, damage induced in metallic window materials

    International Nuclear Information System (INIS)

    Hilscher, D.; Herbach, C.-M.; Jahnke, U.; Tishchenko, V.; Enke, M.; Filges, D.; Goldenbaum, F.; Neef, R.-D.; Nuenighoff, K.; Paul, N.; Schaal, H.; Sterzenbach, G.; Letourneau, A.; Boehm, A.; Galin, J.; Lott, B.; Peghaire, A.; Pienkowski, L.

    2001-01-01

    Production cross-sections for neutrons and charged particles as well as excitation energy distributions in spallation reactions were measured recently by the NESSI-collaboration and have been employed to test different intra nuclear cascade models and the subsequent evaporation. The INCL/GEMINI code, which describes best the experimental data has been employed to calculate the damage cross-sections in Fe and Ta as well as the He/dpa ratio as a function of proton energy. For the same amount of neutron production in a typical target of a spallation neutron source the proton beam induced radiation damage in an Fe window is shown to decrease almost linearly with proton energy. For heavier materials such as Ta a similar decrease of the radiation damage is found only for energies above about 3 GeV

  9. Cross-sections of spallation residues produced in 1A GeV 208Pb on proton reactions

    International Nuclear Information System (INIS)

    Wlazlo, W.; Uniwersytet Jagiellonski, Cracow; Enqvist, T.; Armbruster, P.

    2000-02-01

    Spallation residues produced in 1 GeV per nucleon 208 Pb on proton reactions have been studied using the fragment separator facility at GSI. Isotopic production cross-sections of elements from 61 Pm to 82 Pb have been measured down to 0.1 mb with a high accuracy. The recoil kinetic energies of the produced fragments were also determined. The obtained cross-sections agree with most of the few existing gamma-spectroscopy data. Data are compared with different intranuclear-cascade and evaporation-fission models. Drastic deviations were found for a standard code used in technical applications. (orig.)

  10. Radiation effects concerns at a spallation source

    International Nuclear Information System (INIS)

    Sommer, W.F.

    1990-01-01

    Materials used at spallation neutron sources are exposed to energetic particle and photon radiation. Mechanical and physical properties of these materials are altered; radiation damage on the atomic scale leads to radiation effects on the macroscopic scale. Most notable among mechanical-property radiation effects in metals and metal alloys are changes in tensile strength and ductility, changes in rupture strength, dimensional stability and volumetric swelling, and dimensional changes due to stress-induced creep. Physical properties such as electrical resistivity also are altered. The fission-reactor community has accumulated a good deal of data on material radiation effects. However, when the incident particle energy exceeds 50 MeV or so, a new form of radiation damage ensues; spallation reactions lead to more energetic atom recoils and the subsequent temporal and spatial distribution of point defects is much different from that due to a fission-reactor environment. In addition, spallation reactions cause atomic transmutations with these new atoms representing an impurity in the metal. The higher-energy case is of interest at spallation sources; limited detailed data exist for material performance in this environment. 35 refs., 13 figs., 1 tab

  11. Spallation Neutron Sources For Science And Technology

    International Nuclear Information System (INIS)

    Comsan, M.N.H.

    2011-01-01

    Spallation Neutron Facilities Increasing interest has been noticed in spallation neutron sources (SNS) during the past 20 years. The system includes high current proton accelerator in the GeV region and spallation heavy metal target in the Hg-Bi region. Among high flux currently operating SNSs are: ISIS in UK (1985), SINQ in Switzerland (1996), JSNS in Japan (2008), and SNS in USA (2010). Under construction is the European spallation source (ESS) in Sweden (to be operational in 2020). The intense neutron beams provided by SNSs have the advantage of being of non-reactor origin, are of continuous (SINQ) or pulsed nature. Combined with state-of-the-art neutron instrumentation, they have a diverse potential for both scientific research and diverse applications. Why Neutrons? Neutrons have wavelengths comparable to interatomic spacings (1-5 A) Neutrons have energies comparable to structural and magnetic excitations (1-100 meV) Neutrons are deeply penetrating (bulk samples can be studied) Neutrons are scattered with a strength that varies from element to element (and isotope to isotope) Neutrons have a magnetic moment (study of magnetic materials) Neutrons interact only weakly with matter (theory is easy) Neutron scattering is therefore an ideal probe of magnetic and atomic structures and excitations Neutron Producing Reactions Several nuclear reactions are capable of producing neutrons. However the use of protons minimises the energetic cost of the neutrons produced solid state physics and astrophysics Inelastic neutron scattering

  12. Improvement of spallation reaction simulation codes NMTC/JAERI and NUCLEUS

    International Nuclear Information System (INIS)

    Nishida, T.; Takada, H.; Kanno, I.; Nakahara, Y.

    1990-01-01

    To make evaluations of theoretical models for nuclear spallation reaction, simulation codes are modified and a new mass formula is used to improve the accuracy of Monte Carlo calculations. The following conclusions are made from analyses of calculated distributions of nuclear spallation products. A difference is found between the Cameron's old and the Uno and Yamada's new mass formula, which is due to the difference in the method used to fit their shell energy terms to measured data for selected nuclei and in data themselves. For nuclides with an atomic number larger than 70, mass excesses calculated by the Camerons's mass formula are greater than those by the Uno and Yamada's one, whereas the reverse tendency is seen for ones with atomic numbers smaller than 70. Analysis shows that the distributions of produced nuclei have patterns that appear natural from a physical point of view when artificial restrictions are removed in counting the nuclide production events. The new mass formula can reproduce fairly well the experimental product yield distributions, especially in the neutron excess side. It is also found that the old mass formula gives lower estimations for the number of produced nuclei than the new one, especially in the nuclide region far from the beta stable line. (N.K.)

  13. Spallator - accelerator breeder

    International Nuclear Information System (INIS)

    Steinberg, M.

    1985-01-01

    The concept involves the use of spallation neutrons produced by interaction of a high energy proton (1 to 2 GeV) from a linear accelerator (LINAC) with a heavy metal target (uranium). The principal spallator concept is based on generating fissile fuel for use in LWR nuclear power plants. The spallator functions in conjunction with a reprocessing plant to regenerate and produce the Pu-239 or U-233 for fabrication into fresh LWR reactor fuel elements. Advances in proton accelerator technology has provided a solid base for predicting performance and optimizing the design of a reliable, continuous wave, high-current LINAC required by a fissile fuel production machine

  14. Measurements of activation reaction rate distributions on a mercury target bombarded with high-energy protons at AGS

    International Nuclear Information System (INIS)

    Takada, Hiroshi; Kasugai, Yoshimi; Nakashima, Hiroshi; Ikeda, Yujiro; Jerde, Eric; Glasgow, David

    2000-02-01

    A neutronics experiment was carried out using a thick mercury target at the Alternating Gradient Synchrotron (AGS) facility of Brookhaven National Laboratory in a framework of the ASTE (AGS Spallation Target Experiment) collaboration. Reaction rate distributions around the target were measured by the activation technique at incident proton energies of 1.6, 12 and 24 GeV. Various activation detectors such as the 115 In(n,n') 115m In, 93 Nb(n,2n) 92m Nb, and 209 Bi(n,xn) reactions with threshold energies ranging from 0.3 to 70.5 MeV were employed to obtain the reaction rate data for estimating spallation source neutron characteristics of the mercury target. It was found from the measured 115 In(n,n') 115m In reaction rate distribution that the number of leakage neutrons becomes maximum at about 11 cm from the top of hemisphere of the mercury target for the 1.6-GeV proton incidence and the peak position moves towards forward direction with increase of the incident proton energy. The similar result was observed in the reaction rate distributions of other activation detectors. The experimental procedures and a full set of experimental data in numerical form are summarized in this report. (author)

  15. The future plan for the applications of RI produced in the proton-induced spallation-reaction

    Energy Technology Data Exchange (ETDEWEB)

    Ikezoe, Hiroshi [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

    1997-07-01

    A plan of research facilities (transmutations of minor actinides and neutron scattering for material and life sciences) has been proposed in JAERI. This plan is based on a proton lineac with an energy of 1.5 GeV and a beam current of several mA. Among these facilities, we are planning to accelerate neutron-rich radioactive nuclei (RI) produced in the fission and spallation reactions of thorium or uranium bombarded by the intense high energy proton beams. The RI produced in an ion source are separated by a high resolution isotope separator and their charge states are changed to be negative to inject into the existing tandem-booster accelerator. Main purpose of this plan is to study the nuclear and chemical properties of neutron rich transactinium elements not yet synthesized and the nuclear structures of neutron rich nuclei far from the nuclear stability line. (author)

  16. An update on measurements of helium-production reactions with a spallation neutron source

    International Nuclear Information System (INIS)

    Haight, R.C.; Bateman, F.B.; Chadwick, M.B.

    1995-01-01

    This report gives the status, updated since the last Research Coordination Meeting, of alpha-particle production cross sections, emission spectra and angular distributions which we are measuring at the spallation source of fast neutrons at the Los Alamos Meson Physics Facility (LAMPF). Detectors at angles of 30, 60, 90 and 135 degrees are used to identify alpha particles, measure their energy spectra, and indicate the time-of-flight, and hence the energy, of the neutrons inducing the reaction. The useful neutron energy ranges from less than 1 MeV to approximately 50 MeV for the present experimental setup. Targets under study at present include C, N, 0, 27 Al, Si, 51 V, 56 Fe, 59 CO, 58,60 Ni, 89 Y and 93 Nb. Data for 59 Co have been re-analyzed. The results illustrate the capabilities of the approach, agreement with literature values, and comparisons with nuclear reaction model calculations

  17. An update on measurements of helium-production reactions with a spallation neutron source

    Energy Technology Data Exchange (ETDEWEB)

    Haight, R.C.; Bateman, F.B.; Chadwick, M.B. [and others

    1995-10-01

    This report gives the status, updated since the last Research Coordination Meeting, of alpha-particle production cross sections, emission spectra and angular distributions which we are measuring at the spallation source of fast neutrons at the Los Alamos Meson Physics Facility (LAMPF). Detectors at angles of 30, 60, 90 and 135{degrees} are used to identify alpha particles, measure their energy spectra, and indicate the time-of-flight, and hence the energy, of the neutrons inducing the reaction. The useful neutron energy ranges from less than 1 MeV to approximately 50 MeV for the present experimental setup. Targets under study at present include C, N, 0, {sup 27}Al, Si, {sup 51}V, {sup 56}Fe, {sup 59}CO, {sup 58,60}Ni, {sup 89}Y and {sup 93}Nb. Data for {sup 59}Co have been re-analyzed. The results illustrate the capabilities of the approach, agreement with literature values, and comparisons with nuclear reaction model calculations.

  18. Nuclear chemistry research of high-energy nuclear reactions at Carnegie-Mellon University, 1961--1977. Summary report

    International Nuclear Information System (INIS)

    Caretto, A.A. Jr.

    1977-11-01

    The activities and the results of research in the study of high energy nuclear reactions carried out at Carnegie Institute of Technology from 1957 to 1967 and at Carnegie-Mellon University from 1967 to 1977 are summarized. A complete list of all publications, doctoral dissertations, and reports resulting from the research of this project is also included. A major part of the report is a review of the research activities and results. The objective of the research of this project was the study of reactions initiated by projectiles of energy above about 100 MeV. The main effort was the investigation of simple nuclear reactions with the objective to deduce reaction mechanisms. These reactions were also used as probes to determine the nuclear structure of the target. In addition, a number of studies of spallation reactions were undertaken which included the determination of excitation functions and recoil properties. Recent research activities which have involved the study of pion induced reactions as well as reactions initiated by heavy ions is also discussed

  19. Structural materials for fusion and spallation sources

    International Nuclear Information System (INIS)

    Cottrell, G.A.; Baker, L.J.

    2003-01-01

    Experimental investigation of neutron-induced irradiation damage in structural materials is fundamental to the development of magnetic confinement fusion. Proposals for the testing of candidate materials are described, indicating that a period of at least 10 years will elapse before a suitable high neutron fluence fusion test facility becomes available. In this circumstance, the possibility that neutron spallation sources could be exploited to shorten the time-scale of fusion materials development is attractive. Although fusion displacement and transmutation reaction rates can be replicated in spallation sources, there are significant differences arising from the harder neutron spectra and the presence of energetic protons. These differences, including higher energy PKA, electron heating effects, transmutation rates and pulsing are described and their consequences discussed, together with the concomitant development of theoretical models, needed to understand the effects. It is concluded that spallation source experiments could make a significant contribution to the database required for the validation of theoretical models, and hence reduce the time scale of fusion materials development

  20. Modelling of the spallation reaction: analysis and testing of nuclear models; Simulation de la spallation: analyse et test des modeles nucleaires

    Energy Technology Data Exchange (ETDEWEB)

    Toccoli, C

    2000-04-03

    The spallation reaction is considered as a 2-step process. First a very quick stage (10{sup -22}, 10{sup -29} s) which corresponds to the individual interaction between the incident projectile and nucleons, this interaction is followed by a series of nucleon-nucleon collisions (intranuclear cascade) during which fast particles are emitted, the nucleus is left in a strongly excited level. Secondly a slower stage (10{sup -18}, 10{sup -19} s) during which the nucleus is expected to de-excite completely. This de-excitation is performed by evaporation of light particles (n, p, d, t, {sup 3}He, {sup 4}He) or/and fission or/and fragmentation. The HETC code has been designed to simulate spallation reactions, this simulation is based on the 2-steps process and on several models of intranuclear cascades (Bertini model, Cugnon model, Helder Duarte model), the evaporation model relies on the statistical theory of Weiskopf-Ewing. The purpose of this work is to evaluate the ability of the HETC code to predict experimental results. A methodology about the comparison of relevant experimental data with results of calculation is presented and a preliminary estimation of the systematic error of the HETC code is proposed. The main problem of cascade models originates in the difficulty of simulating inelastic nucleon-nucleon collisions, the emission of pions is over-estimated and corresponding differential spectra are badly reproduced. The inaccuracy of cascade models has a great impact to determine the excited level of the nucleus at the end of the first step and indirectly on the distribution of final residual nuclei. The test of the evaporation model has shown that the emission of high energy light particles is under-estimated. (A.C.)

  1. Investigation of the energy correlations of spallation neutrons by the MCNPX code

    International Nuclear Information System (INIS)

    Szieberth, Mate; Radocz, Gabor

    2011-01-01

    Earlier works have suggested that the energy correlations in a spallation source may influence the neutron noise measurements in an ADS. For the calculation of this effect not only the generally known and used one-particle spectrum is needed but also the so-called two particle spectrum, which describes also the energy correlations. Since measured data are not available for the energy distribution of the neutrons from a single spallation event the physical models of the MCNPX code have been used to investigate the effect. The calculational model has been successfully validated with measurements of the number distribution of spallation neutrons. The simulated one- and two-particle energy distributions and spectra proved that the energy correlations exist and have an important effect in low multiplicity spallation events and in thin targets. On the other hand for thick targets this effect appears negligible and the factorization of the two-particle spectrum seems an acceptable approximation. Further investigations are in hand to quantify the actual effect of the energy correlations on the neutron noise measurements. (author)

  2. Measurements of activation reaction rate distributions on a mercury target bombarded with high-energy protons at AGS

    Energy Technology Data Exchange (ETDEWEB)

    Takada, Hiroshi; Kasugai, Yoshimi; Nakashima, Hiroshi; Ikeda, Yujiro [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment; Ino, Takashi; Kawai, Masayoshi [High Energy Accelerator Research Organization, Tsukuba, Ibaraki (Japan); Jerde, Eric; Glasgow, David [Oak Ridge National Laboratory, Oak Ridge, TN (United States)

    2000-02-01

    A neutronics experiment was carried out using a thick mercury target at the Alternating Gradient Synchrotron (AGS) facility of Brookhaven National Laboratory in a framework of the ASTE (AGS Spallation Target Experiment) collaboration. Reaction rate distributions around the target were measured by the activation technique at incident proton energies of 1.6, 12 and 24 GeV. Various activation detectors such as the {sup 115}In(n,n'){sup 115m}In, {sup 93}Nb(n,2n){sup 92m}Nb, and {sup 209}Bi(n,xn) reactions with threshold energies ranging from 0.3 to 70.5 MeV were employed to obtain the reaction rate data for estimating spallation source neutron characteristics of the mercury target. It was found from the measured {sup 115}In(n,n'){sup 115m}In reaction rate distribution that the number of leakage neutrons becomes maximum at about 11 cm from the top of hemisphere of the mercury target for the 1.6-GeV proton incidence and the peak position moves towards forward direction with increase of the incident proton energy. The similar result was observed in the reaction rate distributions of other activation detectors. The experimental procedures and a full set of experimental data in numerical form are summarized in this report. (author)

  3. Outline of spallation neutron source engineering

    Energy Technology Data Exchange (ETDEWEB)

    Watanabe, Noboru [Center for Neutron Science, Tokai Research Establishment, Japan Atomic Energy Research Institute, Tokai, Ibaraki (Japan)

    2001-01-01

    Slow neutrons such as cold and thermal neutrons are unique probes which can determine structures and dynamics of condensed matter in atomic scale. The neutron scattering technique is indispensable not only for basic sciences such as condensed matter research and life science, but also for basic industrial technology in 21 century. It is believed that to survive in the science-technology competition in 21 century would be almost impossible without neutron scattering. However, the intensity of neutrons presently available is much lower than synchrotron radiation sources, etc. Thus, R and D of intense neutron sources become most important. The High-Intensity Proton Accelerator Project is now being promoted jointly by Japan Atomic Energy Research Institute and High Energy Accelerator Research Organization, but there has so far been no good text which covers all the aspects of pulsed spallation neutron sources. The present review was prepare aiming at giving a better understanding on pulsed spallation neutron sources not only to neutron source researchers but also more widely to neutron scattering researchers and accelerator scientists in this field. The contents involve, starting from what is neutron scattering and what neutrons are necessary for neutron scattering, what is the spallation reaction, how to produce neutrons required for neutron scattering more efficiently, target-moderator-reflector neutronics and its engineering, shielding, target station, material issues, etc. The author have engaged in R and D of pulsed apallation neutron sources and neutron scattering research using them over 30 years. The present review is prepared based on the author's experiences with useful information obtained through ICANS collaboration and recent data from the JSNS (Japanese Spallation Neutron Source) design team. (author)

  4. Studies of short-lived products of spallation fission reactions at TRIUMF

    CERN Document Server

    Bischoff, G; D'Auria, J M; Dautet, H; Lee, J K P; Pate, B D; Wiesehahn, W

    1976-01-01

    The gas-jet recoil transport technique has been used to transport products from spallation and fission reactions from a target chamber to a shielded location for nuclear spectroscopic studies. These involve X- beta - gamma coincidence measurements and (shortly) time- of-flight mass spectroscopy. It has been deduced that the proton beam at present intensities has no appreciable effect on the ability of ethylene and other cluster-producing gases to transport radioactivity. Preliminary results will be presented for shortlived fission products from uranium, and for spallation products of iodine and argon. The latter were obtained from the bombardment of gas and aerosol targets mixed with the transporting gas in the target chamber, which appears to be a generally useful technique.

  5. Evaluation of the transmutation of transuranic using neutrons spectrum from the spallation reaction

    Energy Technology Data Exchange (ETDEWEB)

    Gilberti, Mauricio; Pereira, Claubia, E-mail: mgilber@eletronuclear.gov.br [Eletrobras Termonuclear S.A. (ELETRONUCLEAR), Angra dos Reis, RJ (Brazil); Veloso, Maria A. Fortini, E-mail: claubia@nuclear.ufmg.br [Universidade Federal de Minas Gerais (UFMG), Belo Horizante, MG (Brazil). Dept. de Engenharia Nuclear

    2013-07-01

    The transmutation of transuranic was analyzed by simulating the neutron flux from different spallation sources across arrays of fissile material with isotopic composition PWR reprocessing. A simplified model of Accelerator-Driven Systems (ADS) containing target, moderator graphite, lead-bismuth coolant or sodium coolant, is used. The simulation was made using the particles transport code MCNPX 2.6.0 which allowed to evaluate the rate of transmutation of actinides (Np, Pu, Am, and Cm) at different locations in the system. The objective of the study is to evaluate which the behavior and influences the spectrum of the spallation in the transmutation without the contribution or interference of multiplier, medium subcritical, which would add the contribution of fission neutrons generated, thus interfering in the analysis. The arrangement enable to infer the influence of hardened neutron flux from the spallation reaction in the transmutation, the results show that this is independent of the target material chosen, and the spectrum of spallation has a negligible importance compared to the influence of moderation and scattering generated by the coolant or moderator used. (author)

  6. Evaluation of the transmutation of transuranic using neutrons spectrum from the spallation reaction

    International Nuclear Information System (INIS)

    Gilberti, Mauricio; Pereira, Claubia; Veloso, Maria A. Fortini

    2013-01-01

    The transmutation of transuranic was analyzed by simulating the neutron flux from different spallation sources across arrays of fissile material with isotopic composition PWR reprocessing. A simplified model of Accelerator-Driven Systems (ADS) containing target, moderator graphite, lead-bismuth coolant or sodium coolant, is used. The simulation was made using the particles transport code MCNPX 2.6.0 which allowed to evaluate the rate of transmutation of actinides (Np, Pu, Am, and Cm) at different locations in the system. The objective of the study is to evaluate which the behavior and influences the spectrum of the spallation in the transmutation without the contribution or interference of multiplier, medium subcritical, which would add the contribution of fission neutrons generated, thus interfering in the analysis. The arrangement enable to infer the influence of hardened neutron flux from the spallation reaction in the transmutation, the results show that this is independent of the target material chosen, and the spectrum of spallation has a negligible importance compared to the influence of moderation and scattering generated by the coolant or moderator used. (author)

  7. High energy neutron radiography

    International Nuclear Information System (INIS)

    Gavron, A.; Morley, K.; Morris, C.; Seestrom, S.; Ullmann, J.; Yates, G.; Zumbro, J.

    1996-01-01

    High-energy spallation neutron sources are now being considered in the US and elsewhere as a replacement for neutron beams produced by reactors. High-energy and high intensity neutron beams, produced by unmoderated spallation sources, open potential new vistas of neutron radiography. The authors discuss the basic advantages and disadvantages of high-energy neutron radiography, and consider some experimental results obtained at the Weapons Neutron Research (WNR) facility at Los Alamos

  8. Quantum molecular dynamics approach to estimate spallation yield ...

    Indian Academy of Sciences (India)

    Consequently, the need for reliable data to design and construct spallation neutron sources has prompted ... A major disadvantage of the QMD code .... have estimated the average neutron multiplicities per primary reaction and kinetic energy.

  9. Detection of supernova neutrinos at spallation neutron sources

    Science.gov (United States)

    Huang, Ming-Yang; Guo, Xin-Heng; Young, Bing-Lin

    2016-07-01

    After considering supernova shock effects, Mikheyev-Smirnov-Wolfenstein effects, neutrino collective effects, and Earth matter effects, the detection of supernova neutrinos at the China Spallation Neutron Source is studied and the expected numbers of different flavor supernova neutrinos observed through various reaction channels are calculated with the neutrino energy spectra described by the Fermi-Dirac distribution and the “beta fit” distribution respectively. Furthermore, the numerical calculation method of supernova neutrino detection on Earth is applied to some other spallation neutron sources, and the total expected numbers of supernova neutrinos observed through different reactions channels are given. Supported by National Natural Science Foundation of China (11205185, 11175020, 11275025, 11575023)

  10. Study of the spallation residues in the reaction Au (800 MeV/nucleon) + p; Etude des residus de spallation dans la reaction Au (800 MeV par nucleon) + p

    Energy Technology Data Exchange (ETDEWEB)

    Mustapha, Brahim [Inst. de Physique Nucleaire, Paris-11 Univ., 91 - Orsay (France)

    1999-09-09

    As a neutron source, the spallation reaction is of importance for different fields of research and for a possible hybrid reactor. The study of spallation residues, their cross sections and their energetic properties, is necessary for such applications and for a better understanding of this process. Several studies of spallation products were done using spectroscopic methods. Only radioactive nuclides were detected. Aiming at a more precise measurement, covering the whole range of spallation residues, this study was done using the reverse kinematics method. A liquid hydrogen target was irradiated by an 800 MeV/nucleon gold beam. The produced nuclei were detected in flight before any radioactive decay with about 10% precision. Independent cross section were then obtained. Velocity distributions were completely reconstructed. In their present forms, the theoretical calculations based upon the two-step model, 'intra-nuclear cascade' + 'evaporation', are unable to reproduce the whole set of experimental aspects. An inter-comparison using different INC/EVA combinations permitted to identify the more significant points in these calculations. The important behaviour of this codes were examined. Due to compensation effects between both steps, cascade and evaporation, this study did not lead to a definite conclusion. (author)

  11. Measurement of the spallation reaction 56Fe+p in inverse kinematics

    International Nuclear Information System (INIS)

    Boehmer, M.

    2006-01-01

    In this work the spallation reaction 56 Fe+p was investigated in inverse kinematics with regard to complete identification of the heavy residues. A ring imaging Cerenkov counter was used for velocity measurements in the experimental setup located at GSI in Darmstadt. A new fast readout electronic was developed and has been operated successfully in the experiment. Momentum reconstruction was carried out with the ALADiN spectrometer and a new software package written for this purpose. Cross sections and velocity distributions for more than 100 mass separated isotopes could be extracted from the dataset and compared with empirical models and other spallation experiments. The experiences gained in this experiment will be used for systematic improvements in the setup of the new spectrometer R3B at FAIR. (orig.)

  12. High energy particle transport code NMTC/JAM

    International Nuclear Information System (INIS)

    Niita, K.; Takada, H.; Meigo, S.; Ikeda, Y.

    2001-01-01

    We have developed a high energy particle transport code NMTC/JAM, which is an upgrade version of NMTC/JAERI97. The available energy range of NMTC/JAM is, in principle, extended to 200 GeV for nucleons and mesons including the high energy nuclear reaction code JAM for the intra-nuclear cascade part. We compare the calculations by NMTC/JAM code with the experimental data of thin and thick targets for proton induced reactions up to several 10 GeV. The results of NMTC/JAM code show excellent agreement with the experimental data. From these code validation, it is concluded that NMTC/JAM is reliable in neutronics optimization study of the high intense spallation neutron utilization facility. (author)

  13. Spallator: a new option for nuclear power

    Energy Technology Data Exchange (ETDEWEB)

    Steinberg, M.; Grand, P.; Takahashi, H.; Powell, J.R.; Kouts, H.J.

    1983-06-01

    The principles of the spallator reactor are reviewed. Advances in linear accelerator technology allow the design and construction of high current (hundreds of mA) continuous wave high energy (thousands of MeV) proton machines in the near term. Spallation neutronic calculations building on existing experimental results, indicate substantial neutron yields on uranium targets. Spallator target assembly designs based on water cooled reactor technology indicate operable efficient systems. Fuel cycles are presented which supply fissile material to thermal power reactors and reduce fission product waste. Preliminary comparative analysis indicates an economically competitive system in which a single purpose self-sufficient spallator supplies fuel to a number of LWRs. The spallator assures a long-term LWR power reactor economy. International interest in advancing the technology is indicated.

  14. Spallator: a new option for nuclear power

    International Nuclear Information System (INIS)

    Steinberg, M.; Grand, P.; Takahashi, H.; Powell, J.R.; Kouts, H.J.

    1983-06-01

    The principles of the spallator reactor are reviewed. Advances in linear accelerator technology allow the design and construction of high current (hundreds of mA) continuous wave high energy (thousands of MeV) proton machines in the near term. Spallation neutronic calculations building on existing experimental results, indicate substantial neutron yields on uranium targets. Spallator target assembly designs based on water cooled reactor technology indicate operable efficient systems. Fuel cycles are presented which supply fissile material to thermal power reactors and reduce fission product waste. Preliminary comparative analysis indicates an economically competitive system in which a single purpose self-sufficient spallator supplies fuel to a number of LWRs. The spallator assures a long-term LWR power reactor economy. International interest in advancing the technology is indicated

  15. Study of nuclear reactions involving heavy nuclei and intermediate- and high-energy protons and an application in nuclear reactor physics (ADS)

    International Nuclear Information System (INIS)

    Matuoka, Paula Fernanda Toledo

    2016-01-01

    In the present work, intermediate- and high-energy nuclear reactions involving heavy nuclei and protons were studied with the Monte Carlo CRISP (Rio - Ilheus - Sao Paulo Collaboration) model. The most relevant nuclear processes studied were intranuclear cascade and fission-evaporation competition. Preliminary studies showed fair agreement between CRISP model calculation and experimental data of multiplicity of evaporated neutrons (E 20 MeV) were emitted mostly in the intranuclear cascade stage, while evaporation presented larger neutron multiplicity. Fission cross section of 209 mb and spallation cross section of 1788 mb were calculated { both in agreement with experimental data. The fission process resulted in a symmetric mass distribution. Another Monte Carlo code, MCNP, was used for radiation transport in order to understand the role of a spallation neutron source in a ADS (Accelerator Driven System) nuclear reactor. Initially, a PWR reactor was simulated to study the isotopic compositions in spent nuclear fuel. As a rst attempt, a spallation neutron source was adapted to an industrial size nuclear reactor. The results showed no evidence of incineration of transuranic elements and modifications were suggested. (author)

  16. The spallation in reverse kinematics: what for a coincidence measurement?; La spallation en cinematique inverse: pourquoi faire une mesure en coincidence?

    Energy Technology Data Exchange (ETDEWEB)

    Ducret, J.E

    2006-07-15

    The Spaladin installation has been designed to study spallation reactions in reverse kinematics. Furthermore, the heavy and light fragments are detected by coincidence which allows us to get an instantaneous picture of the reaction at a level of accuracy better than that obtained through inclusive measurement. The first part is dedicated to the theoretical description of the different mechanisms involved in the spallation reactions. In the second part we describe the Spaladin installation and report some results on the reaction: Fe{sup 56} + p at an energy of 1 GeV/nucleon. In the third part we expose the performance of the installation through its simulation with the Geant-IV model. We present a study about the sensitivity of the Spaladin installation to theoretical predictions. The fourth part is dedicated to the future experiments that will be performed with the Spaladin installation. (A.C.)

  17. Range calculations for spallation recoils in ThF4 by use of the computer code 'Marlowe'

    International Nuclear Information System (INIS)

    Westmeier, W.; Roessler, K.

    1978-12-01

    The determination of cross sections of spallation reactions requires a knowledge of the target thickness since only the products recoiling from the target are measured and their yield depends on the range. The effective target thickness is a function of the projectile's Z, A and spallation recoil energy and, thus, varies for the individual products. The computer code MARLOWE was used to evaluate energy vs. range curves in the binary collisions approximation. The program was extended to the high energy regime taking into account the stripping of electrons from the projectile and the concomitant changes in the interaction potentials especially for the inelastic part of the collisions. A complementary computer program LATTIC was developed for the parameterization of the lattice description. This code enables the application of MARLOWE to target materials with complicated crystallographic structure. Test calculations for a series of projectile/target combinations showed a reasonable agreement with experimental recoil ranges of Pd, Ag, Os and Ir isotopes from proton induced spallation in Ag, In and Pb targets, respectively. MARLOWE was then applied to calculate product ranges of the 232 Th(p,spall)X-reaction in the ployatomic system ThF 4 . The calculated energy vs. range curves enabled the evaluation of the mean spallation recoil ranges for all possible products, e.g. 170.8 μg/cm 2 for 192 Tl, 115.2 μg/cm 2 for 208 At and 37.1 μg/cm 2 for 223 Ac. (orig.)

  18. Study of the spallation residues in the reaction Au (800 MeV/nucleon) + p

    International Nuclear Information System (INIS)

    Mustapha, Brahim

    1999-01-01

    As a neutron source, the spallation reaction is of importance for different fields of research and for a possible hybrid reactor. The study of spallation residues, their cross sections and their energetic properties, is necessary for such applications and for a better understanding of this process. Several studies of spallation products were done using spectroscopic methods. Only radioactive nuclides were detected. Aiming at a more precise measurement, covering the whole range of spallation residues, this study was done using the reverse kinematics method. A liquid hydrogen target was irradiated by an 800 MeV/nucleon gold beam. The produced nuclei were detected in flight before any radioactive decay with about 10% precision. Independent cross section were then obtained. Velocity distributions were completely reconstructed. In their present forms, the theoretical calculations based upon the two-step model, 'intra-nuclear cascade' + 'evaporation', are unable to reproduce the whole set of experimental aspects. An inter-comparison using different INC/EVA combinations permitted to identify the more significant points in these calculations. The important behaviour of this codes were examined. Due to compensation effects between both steps, cascade and evaporation, this study did not lead to a definite conclusion. (author)

  19. AGS Spallation Target Experiment (ASTE) Collaboration

    International Nuclear Information System (INIS)

    Oyama, Yukio

    1999-01-01

    An experiment on mercury spallation target with high energy proton beam, called as the AGS Spallation Target Experiment (ASTE) Collaboration, has been performed at Alternating Gradient Synchrotron (AGS) of Brookhaven National Laboratory (BNL) in USA, in cooperation among the laboratories in Japan, Europe and USA. The experimental setup, scope and preliminary results are presented in the paper. (author)

  20. Universal odd-even staggering in isotopic fragmentation and spallation cross sections of neutron-rich fragments

    Science.gov (United States)

    Mei, B.; Tu, X. L.; Wang, M.

    2018-04-01

    An evident odd-even staggering (OES) in fragment cross sections has been experimentally observed in many fragmentation and spallation reactions. However, quantitative comparisons of this OES effect in different reaction systems are still scarce for neutron-rich nuclei near the neutron drip line. By employing a third-order difference formula, the magnitudes of this OES in extensive experimental cross sections are systematically investigated for many neutron-rich nuclei with (N -Z ) from 1 to 23 over a broad range of atomic numbers (Z ≈3 -50 ). A comparison of these magnitude values extracted from fragment cross sections measured in different fragmentation and spallation reactions with a large variety of projectile-target combinations over a wide energy range reveals that the OES magnitude is almost independent of the projectile-target combinations and the projectile energy. The weighted average of these OES magnitudes derived from cross sections accurately measured in different reaction systems is adopted as the evaluation value of the OES magnitude. These evaluated OES magnitudes are recommended to be used in fragmentation and spallation models to improve their predictions for fragment cross sections.

  1. The spallation in reverse kinematics: what for a coincidence measurement?

    International Nuclear Information System (INIS)

    Ducret, J.E.

    2006-07-01

    The Spaladin installation has been designed to study spallation reactions in reverse kinematics. Furthermore, the heavy and light fragments are detected by coincidence which allows us to get an instantaneous picture of the reaction at a level of accuracy better than that obtained through inclusive measurement. The first part is dedicated to the theoretical description of the different mechanisms involved in the spallation reactions. In the second part we describe the Spaladin installation and report some results on the reaction: Fe 56 + p at an energy of 1 GeV/nucleon. In the third part we expose the performance of the installation through its simulation with the Geant-IV model. We present a study about the sensitivity of the Spaladin installation to theoretical predictions. The fourth part is dedicated to the future experiments that will be performed with the Spaladin installation. (A.C.)

  2. High energy gamma ray response of liquid scintillator

    International Nuclear Information System (INIS)

    Shigyo, N.; Ishibashi, K.; Matsufuji, N.; Nakamoto, T.; Numajiri, M.

    1994-01-01

    We made the experiment on the spallation reaction. NE213 organic liquid scintillators were used for measuring neutrons and γ rays. To produce the γ ray emission cross section, we used the response functions by EGS4 code. The response functions look like uniform above γ ray energies of 60 MeV. The experimental data of the γ ray emission cross section are different from the data of High Energy Transport Code. (author)

  3. Study of spallation neutrons for the transmutation of long-lived nuclear waste

    International Nuclear Information System (INIS)

    Brochard, F.; Boyard, J.L.; Duchazeaubeneix, J.C.; Durand, J.M.; Faivre, J.C.; Leray, S.; Milleret, G.; Plouin, F.; Whittal, D.M.; Beau, M.; Crespin, S.; Frehaut, J.; Lochard, J.P.; Martinez, E.; Patin, Y.; Petitbon, E.; Sigaud, J.; Legrain, R.; Lepretre, A.; Terrien, Y.; Bacha, F.; Maillard, J.; Silva, J.

    1994-01-01

    With the renewed interest in accelerator-driven systems to transmute long-lived nuclear waste or to produce energy, new requirements for intermediate-energy nuclear data are now emerging. In all these systems, neutrons are produced by spallation reactions induced by around 1 GeV protons on a heavy target. These neutrons then drive a sub-critical blanket in which wastes are burned or energy is produced. A good knowledge of the spallation process (energy and angular distribution of the neutrons) is necessary to design and optimize the target-blanket system: for instance, to determine the best choices of beam energy, of composition and geometry of the target, in order to have the maximum neutron yield at the lowest cost, or to minimize the back-scattering of neutrons to the accelerator. A programme aimed at measuring the double differential cross-sections for the production of spallation neutrons induced by protons and deuterons GeV beams on different targets, is beginning at SATURNE. (authors). 3 refs., 3 figs

  4. Spallation reaction study for fission products in nuclear waste: Cross section measurements for 137Cs, 90Sr and 107Pd on proton and deuteron

    Directory of Open Access Journals (Sweden)

    Wang He

    2017-01-01

    Full Text Available Spallation reactions for the long-lived fission products 137Cs, 90Sr and 107Pd have been studied for the purpose of nuclear waste transmutation. The cross sections on the proton- and deuteron-induced spallation were obtained in inverse kinematics at the RIKEN Radioactive Isotope Beam Factory. Both the target and energy dependences of cross sections have been investigated systematically. and the cross-section differences between the proton and deuteron are found to be larger for lighter fragments. The experimental data are compared with the SPACS semi-empirical parameterization and the PHITS calculations including both the intra-nuclear cascade and evaporation processes.

  5. Study of nuclear reactions involving heavy nuclei and intermediate- and high-energy protons and an application in nuclear reactor physics (ADS); Estudo das reacoes nucleares envolvendo nucleos pesados e protons a energias intermediarias e altas de uma aplicacao em fisica de reatores nucleares (ADS)

    Energy Technology Data Exchange (ETDEWEB)

    Matuoka, Paula Fernanda Toledo

    2016-07-01

    In the present work, intermediate- and high-energy nuclear reactions involving heavy nuclei and protons were studied with the Monte Carlo CRISP (Rio - Ilheus - Sao Paulo Collaboration) model. The most relevant nuclear processes studied were intranuclear cascade and fission-evaporation competition. Preliminary studies showed fair agreement between CRISP model calculation and experimental data of multiplicity of evaporated neutrons (E < 20 MeV) from the p(1200 MeV) + {sup 208}Pb reaction and of spallation residues from the p(1000 MeV) + {sup 208}Pb reaction. The investigation of neutron multiplicity from proton-induced fission of {sup 232}Th up to 85 MeV showed that it was being overestimated by CRISP model; on the other hand, fission cross section were being underestimated. This behavior is due to limitations of the intranuclear cascade model for low-energies (around 50 MeV). The p(1200 MeV) + {sup 208}Pb reaction was selected for the study of a spallation neutron source. High-energy neutrons (E > 20 MeV) were emitted mostly in the intranuclear cascade stage, while evaporation presented larger neutron multiplicity. Fission cross section of 209 mb and spallation cross section of 1788 mb were calculated both in agreement with experimental data. The fission process resulted in a symmetric mass distribution. Another Monte Carlo code, MCNP, was used for radiation transport in order to understand the role of a spallation neutron source in a ADS (Accelerator Driven System) nuclear reactor. Initially, a PWR reactor was simulated to study the isotopic compositions in spent nuclear fuel. As a rst attempt, a spallation neutron source was adapted to an industrial size nuclear reactor. The results showed no evidence of incineration of transuranic elements and modifications were suggested. (author)

  6. Development of nuclear design criteria for neutron spallation sources

    Energy Technology Data Exchange (ETDEWEB)

    Sordo, F.; Abanades, A. [E.T.S. Industriales, Madrid Polytechnic University, UPM, J.Gutierrez Abascal, 2 -28006 Madrid (Spain)

    2008-07-01

    Spallation neutron sources allow obtaining high neutronic flux for many scientific and industrial applications. In recent years, several proposals have been made about its use, notably the European Spallation Source (ESS), the Japanese Spallation Source (JSNS) and the projects of Accelerator-Driven Subcritical reactors (ADS), particularly in the framework of EURATOM programs. Given their interest, it seems necessary to establish adequate design basis for guiding the engineering analysis and construction projects of this kind of installations. In this sense, all works done so far seek to obtain particular solutions to a particular design, but there has not been any general development to set up an engineering methodology in this field. In the integral design of a spallation source, all relevant physical processes that may influence its behaviour must be taken into account. Neutronic aspects (emitted neutrons and their spectrum, generation performance..), thermomechanical (energy deposition, cooling conditions, stress distribution..), radiological (spallation waste activity, activation reactions and residual heat) and material properties alteration due to irradiation (atomic displacements and gas generation) must all be considered. After analysing in a systematic manner the different options available in scientific literature, the main objective of this thesis was established as making a significant contribution to determine the limiting factors of the main aspects of spallation sources, its application range and the criteria for choosing optimal materials. To achieve this goal, a series of general simulations have been completed, covering all the relevant physical processes in the neutronic and thermal-mechanical field. Finally, the obtained criteria have been applied to the particular case of the design of the spallation source of subcritical reactors PDX-ADS and XT-ADS. These two designs, developed under the European R and D Framework Program, represent nowadays

  7. Development of nuclear design criteria for neutron spallation sources

    International Nuclear Information System (INIS)

    Sordo, F.; Abanades, A.

    2008-01-01

    Spallation neutron sources allow obtaining high neutronic flux for many scientific and industrial applications. In recent years, several proposals have been made about its use, notably the European Spallation Source (ESS), the Japanese Spallation Source (JSNS) and the projects of Accelerator-Driven Subcritical reactors (ADS), particularly in the framework of EURATOM programs. Given their interest, it seems necessary to establish adequate design basis for guiding the engineering analysis and construction projects of this kind of installations. In this sense, all works done so far seek to obtain particular solutions to a particular design, but there has not been any general development to set up an engineering methodology in this field. In the integral design of a spallation source, all relevant physical processes that may influence its behaviour must be taken into account. Neutronic aspects (emitted neutrons and their spectrum, generation performance..), thermomechanical (energy deposition, cooling conditions, stress distribution..), radiological (spallation waste activity, activation reactions and residual heat) and material properties alteration due to irradiation (atomic displacements and gas generation) must all be considered. After analysing in a systematic manner the different options available in scientific literature, the main objective of this thesis was established as making a significant contribution to determine the limiting factors of the main aspects of spallation sources, its application range and the criteria for choosing optimal materials. To achieve this goal, a series of general simulations have been completed, covering all the relevant physical processes in the neutronic and thermal-mechanical field. Finally, the obtained criteria have been applied to the particular case of the design of the spallation source of subcritical reactors PDX-ADS and XT-ADS. These two designs, developed under the European R and D Framework Program, represent nowadays

  8. On spallation and fragmentation of heavy ions at intermediate energies

    International Nuclear Information System (INIS)

    Musulmanbekov, G.; Al-Haidary, A.

    2002-01-01

    A new code for simulation of spallation and (multi)fragmentation of nuclei in proton and nucleus induced collisions at intermediate and high energies is developed. The code is a combination of modified intranuclear cascade model with traditional fission - evaporation part and multifragmentation part based on lattice representation of nuclear structure and percolation approach. The production of s-wave resonances and formation time concept included into standard intranuclear cascade code provides correct calculation of excitation energy of residues. This modified cascade code served as a bridge between low and high energy model descriptions of nucleus-nucleus collisions. A good agreement with experiments has been obtained for multiparticle production at intermediate and relatively high energies. Nuclear structure of colliding nuclei is represented as face centered cubic lattice. This representation, being isomorphic to the shell model of nuclear structure, allows to apply percolation approach for nuclear fragmentation. The offered percolation model includes both site and bond percolation. Broken sites represent holes left by nucleons knocked out at cascade state. Therefore, in the first cascade stage mutual rescattering of the colliding nuclei results in knocking some nucleons out of them. After this fast stage paltrily destruct and excited residues remain. On the second stage residual nuclei either evaporate nucleons and light nuclei up to alpha-particles or fragment into pieces with intermediate masses. The choice depends on residue's destruction degree. At low excitation energy and small destruction of the residue the evaporation and fission mechanisms are preferable. The more excitation energy and destruction the more probability of (multi)fragmentation process. Moreover, the more destruction degree of the residual the more the site percolation probability. It is concluded, that at low and intermediate excitation energies the fragmentation of nuclei is slow

  9. Spallation target-moderator-reflector studies at the Weapons Neutron Research facility

    International Nuclear Information System (INIS)

    Russell, G.J.; Gilmore, J.S.; Prael, S.D.; Robinson, H.; Howe, S.D.

    1980-01-01

    Basic neutronics data, initiated by 800-MeV proton spallation reactions, are important to spallation neutron source development and electronuclear fuel production. Angle-dependent and energy-dependent neutron production cross sections, energy-dependent and total neutron yields, thermal and epithermal neutron surface and beam fluxes, and fertile-to-fissile conversion ratios are being measured. The measurements are being done at the Weapons Neutron Research facility on a variety of targets and target-moderator-reflector configurations. The experiments are relevant to the above applications, and provide data to validate computer codes. Preliminary results are presented and compared to calculated predictions. 13 figures

  10. Spallation neutron spectra measured at Saturne

    International Nuclear Information System (INIS)

    Boyard, J.L.; Bouyer, P.; Brochard, F.; Duchazeaubeneix, J.C.; Durand, J.M.; Leray, S.; Milleret, G.; Plouin, F.; Uematsu, M.; Whittal, D.M.; Martinez, E.; Beau, M.; Boue, F.; Crespin, S.; Drake, D.; Frehaut, J.; Lochard, J.P.; Patin, Y.; Petibon, E.; Legrain, R.; Terrien, Y.

    1995-01-01

    Good knowledge of spallation reactions is necessary to design accelerator-based transmutation systems. An extensive program has begun at Saturne to measure energy and angular distributions of neutrons produced by incident protons or deuterons of up to 2 GeV on several thin targets. Our measurements will extend the available data to higher energies than the present limit of 800 MeV enabling improvements to the codes which are sometimes in poor agreement with the data. (Authors). 7 refs., 7 figs

  11. Neutronics of pulsed spallation neutron sources

    International Nuclear Information System (INIS)

    Watanabe, Noboru

    2003-01-01

    Various topics and issues on the neutronics of pulsed spallation neutron sources, mainly for neutron scattering experiments, are reviewed to give a wide circle of readers a better understanding of these sources in order to achieve a high neutronic performance. Starting from what neutrons are needed, what the spallation reaction is and how to produce slow-neutrons more efficiently, the outline of the target and moderator neutronics are explained. Various efforts with some new concepts or ideas have already been devoted to obtaining the highest possible slow-neutron intensity with desired pulse characteristics. This paper also reviews the recent progress of such efforts, mainly focused on moderator neutronics, since moderators are the final devices of a neutron source, which determine the source performance. Various governing parameters for neutron-pulse characteristics such as material issues, geometrical parameters (shape and dimensions), the target-moderator coupling scheme, the ortho-para-hydrogen ratio, poisoning, etc are discussed, aiming at a high performance pulsed spallation source

  12. Spallation reaction study for fission products in nuclear waste: Cross section measurements for {sup 137}Cs and {sup 90}Sr on proton and deuteron

    Energy Technology Data Exchange (ETDEWEB)

    Wang, H., E-mail: wanghe@ribf.riken.jp [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Otsu, H.; Sakurai, H.; Ahn, D.S. [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Aikawa, M. [Faculty of Science, Hokkaido University, Sapporo 060-0810 (Japan); Doornenbal, P.; Fukuda, N.; Isobe, T. [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Kawakami, S. [Department of Applied Physics, University of Miyazaki, Miyazaki 889-2192 (Japan); Koyama, S. [Department of Physics, University of Tokyo, 7-3-1 Hongo, Bunkyo, Tokyo 113-0033 (Japan); Kubo, T.; Kubono, S.; Lorusso, G. [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Maeda, Y. [Department of Applied Physics, University of Miyazaki, Miyazaki 889-2192 (Japan); Makinaga, A. [Graduate School of Medicine, Hokkaido University, North-14, West-5, Kita-ku, Sapporo 060-8648 (Japan); Momiyama, S. [Department of Physics, University of Tokyo, 7-3-1 Hongo, Bunkyo, Tokyo 113-0033 (Japan); Nakano, K. [Department of Advanced Energy Engineering Science, Kyushu University, Kasuga, Fukuoka 816-8580 (Japan); Niikura, M. [Department of Physics, University of Tokyo, 7-3-1 Hongo, Bunkyo, Tokyo 113-0033 (Japan); Shiga, Y. [Department of Physics, Rikkyo University, 3-34-1 Nishi-Ikebukuro, Toshima, Tokyo 171-8501 (Japan); RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Söderström, P.-A. [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); and others

    2016-03-10

    We have studied spallation reactions for the fission products {sup 137}Cs and {sup 90}Sr for the purpose of nuclear waste transmutation. The spallation cross sections on the proton and deuteron were obtained in inverse kinematics for the first time using secondary beams of {sup 137}Cs and {sup 90}Sr at 185 MeV/nucleon at the RIKEN Radioactive Isotope Beam Factory. The target dependence has been investigated systematically, and the cross-section differences between the proton and deuteron are found to be larger for lighter spallation products. The experimental data are compared with the PHITS calculation, which includes cascade and evaporation processes. Our results suggest that both proton- and deuteron-induced spallation reactions are promising mechanisms for the transmutation of radioactive fission products.

  13. Spallation radiation damage and dosimetry for accelerator transmutation of waste applications

    International Nuclear Information System (INIS)

    Wechsler, M.S.; Lin, C.

    1993-01-01

    Proposals are currently being made for systems to treat radioactive waste based on the use of accelerator-driven neutron sources. A linear proton accelerator with energies as high as 1600 MeV and currents up to 250 ma are anticipated for the driver. The neutron fluxes may reach up to 10 20 neutrons/m 2 s as generated by the spallation reactions that occur when the protons strike target materials. Calculations are described to determine radiation fluxes and flux spectra inherent in such systems and to estimate likely radiation effects on system components. The calculations use LAHET, a Monte Carlo high-energy transport code, and MCNP, a generalized-geometry, coupled neutron-photon Monte Carlo transport code. Cross sections for displacement and helium production are presented for spallation neutrons of energies from 21 MeV to 1600 MeV for Inconel 718 (Ni plus 18.5, 18.5, 5.1, and 3 wt % of Cr, Fe, Nb, and Mo, respectively), an alloy that is used for the proton beam entry window in several accelerators. In addition, results for this alloy are presented for the primary knocked-on atom (PKA) spectrum and the transmutation yield for 1600 MeV incident neutrons

  14. Calculation of the spallation product distribution in the evaporation process

    International Nuclear Information System (INIS)

    Nishida, T.; Kanno, I.; Nakahara, Y.; Takada, H.

    1989-01-01

    Some investigations are performed for the calculational model of nuclear spallation reaction in the evaporation process. A new version of a spallation reaction simulation code NUCLEUS has been developed by incorporating the newly revised Uno ampersand Yamada's mass formula and extending the counting region of produced nuclei. The differences between the new and original mass formulas are shown in the comparisons of mass excess values. The distributions of spallation products of a uranium target nucleus bombarded by energy (0.38 - 2.9 GeV) protons have been calculated with the new and original versions of NUCLEUS. In the fission component Uno ampersand Yamada's mass formula reproduces the measured data obtained from thin foil experiments significantly better, especially in the neutron excess side, than the combination of the Cameron's mass formula and the mass table compiled by Wapstra, et al., in the original version of NUCLEUS. Discussions are also made on how the mass-yield distribution of products varies dependent on the level density parameter a characterizing the particle evaporation. 16 refs., 7 figs., 1 tab

  15. Calculation of the spallation product distribution in the evaporation process

    International Nuclear Information System (INIS)

    Nishida, T.; Kanno, I.; Nakahara, Y.; Takada, H.

    1989-01-01

    Some investigations are performed for the calculational model of nuclear spallation reaction in the evaporation process. A new version of a spallation reaction simulation code NUCLEUS has been developed by incorporating the newly revised Uno and Yamada's mass formula and extending the counting region of produced nuclei. The differences between the new and original mass formulas are shown in the comparisons of mass excess values. The distributions of spallation products of a uranium target nucleus bombarded by energy (0.38 - 2.9 GeV) protons have been calculated with the new and original versions of NUCLEUS. In the fission component Uno and Yamada's mass formula reproduces the measured data obtained from thin foil experiments significantly better, especially in the neutron excess side, than the combination of the Cameron's mass formula and the mass table compiled by Wapstra, et al., in the original version of NUCLEUS. Discussions are also made on how the mass-yield distribution of products varies dependent on the level density parameter α characterizing the particle evaporation. (author)

  16. Effect of free-particle collisions in high energy proton and pion-induced nuclear reactions

    International Nuclear Information System (INIS)

    Jacob, N.P. Jr.

    1975-07-01

    The effect of free-particle collisions in simple ''knockout'' reactions of the form (a,aN) and in more complex nuclear reactions of the form (a,X) was investigated by using protons and pions. Cross sections for the 48 Ti(p,2p) 47 Sc and the 74 Ge(p,2p) 73 Ga reactions were measured from 0.3 to 4.6 GeV incident energy. The results indicate a rise in (p,2p) cross section for each reaction of about (25 +- 3) percent between the energies 0.3 and 1.0 GeV, and are correlated to a large increase in the total free-particle pp scattering cross sections over the same energy region. Results are compared to previous (p,2p) excitation functions in the GeV energy region and to (p,2p) cross section calculations based on a Monte Carlo intranuclear cascade-evaporation model. Cross section measurements for (π/sup +-/, πN) and other more complex pion-induced spallation reactions were measured for the light target nuclei 14 N, 16 O, and 19 F from 45 to 550 MeV incident pion energy. These measurements indicate a broad peak in the excitation functions for both (π,πN) and (π,X) reactions near 180 MeV incident energy. This corresponds to the large resonances observed in the free-particle π + p and π - p cross sections at the same energy. Striking differences in (π,πN) cross section magnitudes are observed among the light nuclei targets. The experimental cross section ratio sigma(π - ,π - n)/sigma(π + ,πN) at 180 MeV is 1.7 +- 0.2 for all three targets. The experimental results are compared to previous pion and analogous proton-induced reactions, to Monte Carlo intranuclear cascade-evaporation calculations, and to a semi-classical nucleon charge exchange model. (108 references) (auth)

  17. An intranuclear cascade calculation of high-energy heavy-ion interactions

    International Nuclear Information System (INIS)

    Yariv, Y.; Fraenkel, Z.

    1979-01-01

    The intranuclear cascade model of Chen is extended to high-energy reactions between two heavy ions. The results of the calculations are compared with experimental results for the inclusive proton and pion cross sections, two-particle correlations, particle multiplicity distributions and spallation cross section distributions from light ( 12 C+ 12 C) to heavy( 40 Ar + 238 U) projectile-target systems in the laboratory bombarding energy range E/A=250-1000 MeV. The comparison shows that the model is fairly successful in reproducing the various aspects of high-energy reactions between heavy ions. It is also shown that the assumption that high particle multiplicities are indicative of ''central'' (small impact parameter) collisions are well founded for heavy projectile-target systems. (B.G.)

  18. Nuclear chemistry research of high-energy nuclear reactions at Carnegie-Mellon University, 1961--1977. Summary report. [Summaries of research activities at Carnegie-Mellon University

    Energy Technology Data Exchange (ETDEWEB)

    Caretto, A.A. Jr.

    1977-11-01

    The activities and the results of research in the study of high energy nuclear reactions carried out at Carnegie Institute of Technology from 1957 to 1967 and at Carnegie-Mellon University from 1967 to 1977 are summarized. A complete list of all publications, doctoral dissertations, and reports resulting from the research of this project is also included. A major part of the report is a review of the research activities and results. The objective of the research of this project was the study of reactions initiated by projectiles of energy above about 100 MeV. The main effort was the investigation of simple nuclear reactions with the objective to deduce reaction mechanisms. These reactions were also used as probes to determine the nuclear structure of the target. In addition, a number of studies of spallation reactions were undertaken which included the determination of excitation functions and recoil properties. Recent research activities which have involved the study of pion induced reactions as well as reactions initiated by heavy ions is also discussed.

  19. Measurement of activation reaction rate distribution on a mercury target with a lead-reflector and light-water-moderator for high energy proton bombardment using AGS accelerator

    International Nuclear Information System (INIS)

    Kasugai, Yoshimi; Takada, Hiroshi; Meigo, Shin-ichiro

    2001-02-01

    Characteristic of spallation neutrons driven by GeV protons from a mercury target with a lead-reflector and light-water-moderator was studied experimentally using the Alternating Gradient Synchrotron (AGS) facility of Brookhaven National Laboratory in a framework of the ASTE (AGS Spallation Target Experiment) collaboration. Several reaction rates along with the mercury target were measured with the activation method at incident proton energies of 1.94, 12 and 24 GeV. Indium, niobium, aluminum, cobalt, nickel and bismuth were used as activation detectors to cover the threshold energy of between 0.33 and 40.9 MeV. This report summarizes the experimental procedure with all the measured data. (author)

  20. Analysis of the spallation residues and the associated particles in the reaction Fe+p at 1 GeV per nucleon; Analyse des residus de spallation et des particules associees dans la reaction Fe+p a 1 GeV par nucleon

    Energy Technology Data Exchange (ETDEWEB)

    Le Gentil, E

    2006-09-15

    SPALADIN is a new type of spallation experiment that has been carried out at the GSI accelerator facility (Germany) in order to improve the modelling of the spallation reaction. This experiment is based on the coincidence measurement in inverse kinematics of the spallation residues and the de-excitation fragments. This work presents the analysis of Fe{sup 56} + p reaction at 1 GeV per nucleon. Results on cross-sections and heavy residue velocity spectra are compared to previous data and enabled us to characterize the setup. Most of the element production cross-sections have been obtained with an uncertainty below 10 per cent. In the particular case of helium, its production cross-section has been measured to be {sigma}(1 GeV) = (598 {+-} 67) mb. The knowledge of this cross-section is important to assess the irradiation damage undergone by the window separating the accelerator from the target. The study of the de-excitation of the pre-fragment shows that the evaporation of light particles (Z {<=} 2) is the main way of de-excitation whatever the collision centrality. However, the de-excitation through the emission of intermediate mass fragments is observed in 5% of the events and most of these events correspond to a very asymmetric binary breaking. The velocity distributions of light residues (with regards to the mass of the projectile) show a significant disagreement with the average velocities predicted by spallation codes. (A.C.)

  1. Calculations of the main free path on neutron emission cross-section for spallation reaction of target and fuel nuclei

    International Nuclear Information System (INIS)

    Tel, E.; Kisoglu, H. F.; Topaksu, A. K.; Aydin, A.; Kaplan, A.

    2007-01-01

    There are several new technological application fields of fast neutrons such as accelerator-driven incineration/ transmutation of the long-lived radioactive nuclear wastes (in particular transuranium nuclides) to short-lived or stable isotopes by secondary spallation neutrons produced by high-intensity, intermediate-energy, charged-particle beams, prolonged planetary space missions, shielding for particle accelerators. Especially, accelerator driven subcritical systems (ADS) can be used for fission energy production and /or nuclear waste transmutation as well as in the intermediate-energy accelerator driven neutron sources, ions and neutrons with energies beyond 20 MeV, the upper limit of exiting data files that produced for fusion and fission applications. In these systems, the neutron scattering cross sections and emission differential data are very important for reactor neutronics calculations. The transition rate calculation involves the introduction of the parameter of mean free path determines the mean free path of the nucleon in the nuclear matter. This parameter allows an increase in mean free path, with simulation of effect, which is not considered in the calculations, such as conservation of parity and angular momentum in intra nuclear transitions. In this study, we have investigated the multiple preequilibrium matrix element constant from internal transition for Uranium, Thorium, (n,xn) neutron emission spectra. The neutron-emission spectra produced by (n,xn) reactions on nuclei of some target (for spallation) have been calculated. In the calculations, we have used the geometry dependent hybrid model and the cascade exciton model including the effects of the preequilibrium. The pre-equilibrium direct effects have been examined by using full exciton model. All calculated results have been compared with the experimental data. The obtained results have been discussed and compared with the available experimental data and found agreement with each other

  2. Spatial distribution of moderated neutrons along a Pb target irradiated by high-energy protons

    International Nuclear Information System (INIS)

    Fragopoulou, M.; Manolopoulou, M.; Stoulos, S.; Brandt, R.; Westmeier, W.; Kulakov, B.A.; Krivopustov, M.I.; Sosnin, A.N.; Debeauvais, M.; Adloff, J.C.; Zamani Valasiadou, M.

    2006-01-01

    High-energy protons in the range of 0.5-7.4 GeV have irradiated an extended Pb target covered with a paraffin moderator. The moderator was used in order to shift the hard Pb spallation neutron spectrum to lower energies and to increase the transmutation efficiency via (n,γ) reactions. Neutron distributions along and inside the paraffin moderator were measured. An analysis of the experimental results was performed based on particle production by high-energy interactions with heavy targets and neutron spectrum shifting by the paraffin. Conclusions about the spallation neutron production in the target and moderation through the paraffin are presented. The study of the total neutron fluence on the moderator surface as a function of the proton beam energy shows that neutron cost is improved up to 1 GeV. For higher proton beam energies it remains constant with a tendency to decline

  3. Systematics of spallation yields with a four-parameter formula

    International Nuclear Information System (INIS)

    Foshina, M.; Martins, J.B.; Tavares, O.A.P.; Di Napoli, V.

    1982-01-01

    A semi-empirical four-parameter formula is proposed in order to systematize intermediate- and high-energy proton-induced spallation yields of target nuclei covering the 50-100 mass number interval. The measured yields are reproduced by the formula with a degree of accuracy which is comparable with or better than those obtained in previous proton-spallation systematics. The formula predicts reliable values for the most probable mass number of isotopic distributions. For a number of irradiation conditions which may be encountered in practical and physical applications, estimates of proton spallation yields can be obtained by the proposed four-parameter formula with no need of high-speed machines. (M.A.F.) [pt

  4. Delayed neutrons in liquid metal spallation targets

    International Nuclear Information System (INIS)

    Ridikas, D.; Bokov, P.; David, J.C.; Dore, D.; Giacri, M.L.; Van Lauwe, A.; Plukiene, R.; Plukis, A.; Ignatiev, S.; Pankratov, D.

    2003-01-01

    The next generation spallation neutron sources, neutrino factories or RIB production facilities currently being designed and constructed around the world will increase the average proton beam power on target by a few orders of magnitude. Increased proton beam power results in target thermal hydraulic issues leading to new target designs, very often based on flowing liquid metal targets such as Hg, Pb, Pb-Bi. Radioactive nuclides produced in liquid metal targets are transported into hot cells, past electronics, into pumps with radiation sensitive components, etc. Besides the considerable amount of photon activity in the irradiated liquid metal, a significant amount of the delayed neutron precursor activity can be accumulated in the target fluid. The transit time from the front of a liquid metal target into areas, where delayed neutrons may be important, can be as short as a few seconds, well within one half-life of many delayed neutron precursors. Therefore, it is necessary to evaluate the total neutron flux (including delayed neutrons) as a function of time and determine if delayed neutrons contribute significantly to the dose rate. In this study the multi-particle transport code MCNPX combined with the material evolution program CINDER'90 will be used to evaluate the delayed neutron flux and spectra. The following scientific issues will be addressed in this paper: - Modeling of a typical geometry of the liquid metal spallation target; - Predictions of the prompt neutron fluxes, fission fragment and spallation product distributions; - Comparison of the above parameters with existing experimental data; - Time-dependent calculations of delayed neutron precursors; - Neutron flux estimates due to the prompt and delayed neutron emission; - Proposal of an experimental program to measure delayed neutron spectra from high energy spallation-fission reactions. The results of this study should be directly applicable in the design study of the European MegaPie (1 MW

  5. Spallation production of neutron deficient radioisotopes in North America

    International Nuclear Information System (INIS)

    Jamriska, D.J.; Peterson, E.J.; Carty, J.

    1997-01-01

    The United States Department of Energy produces a number of neutron deficient radioisotopes by high energy proton induced spallation reactions in accelerators at Los Alamos National Laboratory in New Mexico and Brookhaven National Laboratory in New York. Research isotopes are also recovered from targets irradiated at TRIUMF in British Columbia, Canada. The radioisotopes recovered are distributed for use in nuclear medicine, environmental research, physics research, and industry worldwide. In addition to the main product line of Sr-82 from either Mo or Rb targets, Cu-67 from ZnO targets, and Ge-68 from RbBr targets, these irradiation facilities also produce some unique isotopes in quantities not available from any other source such as Be-10, Al-26, Mg-28, Si-32, El-44, Fe-52, Gd-248, and Hg-194. We will describe the accelerator irradiation facilities at the Los Alamos and Brookhaven National Laboratories. The high level radiochemical processing facilities at Los Alamos and brief chemical processes from Los Alamos and Brookhaven will be described. Chemical separation techniques have been developed to recover the radioisotopes of interest in both high radiochemical purity and yield and at the same time trying to reduce or eliminate the generation of mixed waste. nearly 75 neutron deficient radioisotopes produced in spallation targets have been produced and distributed to researchers around the world since the inception of the program in 1974

  6. High energy gamma-ray production in nuclear reactions

    International Nuclear Information System (INIS)

    Pinston, J.A.; Nifenecker, H.; Nifenecker, H.

    1989-01-01

    Experimental techniques used to study high energy gamma-ray production in nuclear reactions are reviewed. High energy photon production in nucleus-nucleus collisions is discussed. Semi-classical descriptions of the nucleus-nucleus gamma reactions are introduced. Nucleon-nucleon gamma cross sections are considered, including theoretical aspects and experimental data. High energy gamma ray production in proton-nucleus reactions is explained. Theoretical explanations of photon emission in nucleus-nucleus collisions are treated. The contribution of charged pion currents to photon production is mentioned

  7. Efficiency of an LBE spallation target in an accelerator-driven molten salt subcritical reactor

    Energy Technology Data Exchange (ETDEWEB)

    Bak, Sang-In [Sungkyunkwan University, Suwon (Korea, Republic of); Hong, Seung-Woo [Sungkyunkwan University, Suwon (Korea, Republic of); Kadi, Yacine [CERN, Geneva (Switzerland)

    2016-10-15

    An Accelerator-Driven System (ADS) combined with a subcritical Molten Salt Reactor (MSR) is a type of hybrid reactor originally designed to breed uranium from thorium or to incinerate long-lived minor actinides in nuclear wastes. In an MSR, the salt material is used not only as a nuclear fuel but also as a primary coolant. In addition, this material is used as a target for inducing spallation neutrons in most AD-MSR concepts. A high energy proton beam impinges on a heavy metal target to induce spallation reactions and produces neutrons. Accordingly, a reliable proton accelerator is needed to feed the source neutrons. As ADSs have been criticized for requiring high power accelerators, minimization of beam power is an important aspect of ADS design. A primary concern associated with ADS development is stable high-power accelerators. We therefore studied the neutron source efficiencies of an AD-MSR involving chloride fuels by including a Pb-Bi eutectic (LBE) spallation target. The proton source efficiency and the accelerator beam power required have been studied for an AD-MSR. Adoption of an LBE spallation target induces an increase in proton source efficiencies in comparison to the case without a spallation target. Thus the presence of an efficient spallation target is useful in the reduction of the beam power of an accelerator. Almost 33 % of the beam power can be reduced in comparison to the case without the target for NaCl-Th/{sup 233}U fuel, and about 16 % for NaCl-U/TRU fuel. The beam power amplifications increase by 1.5 times for NaCl-Th/{sup 233}U and 1.2 times for NaCl-U/TRU in comparison with the no target AD-MSR.

  8. Study of the production of residual evaporation nuclei issued from the spallation reaction of uranium-238 by 1 GeV protons; Etude de la production de noyaux residuels d'evaporation issus de la reaction de spallation de l'uranium-238 par des protons a 1 GeV

    Energy Technology Data Exchange (ETDEWEB)

    Taieb, J

    2000-10-01

    The spallation reaction by high energy protons is one of the envisaged nuclear reactions for production of exotic nuclei. We have measured the production of more than 300 different evaporation residues issued by the spallation reaction of Uranium-238 by 1 GeV protons. We used the reverse kinematics technique in order to produce the relativistic nuclei and therefore to be able to detect those nuclides within a very short time, shorter in most cases than the radioactive disintegration period. The achieved nuclear charge and mass resolution are excellent. They allow a good accuracy on the values of the measured cross-sections (10 to 15%). We have observed for the first time the nuclide Actinium-235 obtained consequently to the loss of 3 protons by the projectile. The measured isotopic distribution are strongly influenced by the mechanism of fission which leads to a strong reduction of the production of the heavy neutron deficient isotopes. We have compared our results to some other measurements achieved with radio-chemical methods at a similar energy. We observed a systematic disagreement of about 40%. Some comparison with the available systematics show that those are presently not able to reproduce the data with a reasonable precision. We could also measure the recoil momentum distribution for each studied isotopes. We show that Goldhaber's model agrees very well with the experiment in case. of 'cold' channels where the evaporation of particles never occurs. On the other hand, when the produced pre-fragment is excited the data show that Goldhaber's model does not reproduce.the data showing the limitation of such an approach. We finally tried to reproduce the measurement of evaporation residue cross-section thanks to the coupling of intra-nuclear cascade and statistical evaporation codes. The influence of the fission process is rather important is the system p+U; we therefore had to account for the dynamical aspect of the fission. We also showed

  9. GRAIN-SCALE FAILURE IN THERMAL SPALLATION DRILLING

    Energy Technology Data Exchange (ETDEWEB)

    Walsh, S C; Lomov, I; Roberts, J J

    2012-01-19

    Geothermal power promises clean, renewable, reliable and potentially widely-available energy, but is limited by high initial capital costs. New drilling technologies are required to make geothermal power financially competitive with other energy sources. One potential solution is offered by Thermal Spallation Drilling (TSD) - a novel drilling technique in which small particles (spalls) are released from the rock surface by rapid heating. While TSD has the potential to improve drilling rates of brittle granitic rocks, the coupled thermomechanical processes involved in TSD are poorly described, making system control and optimization difficult for this drilling technology. In this paper, we discuss results from a new modeling effort investigating thermal spallation drilling. In particular, we describe an explicit model that simulates the grain-scale mechanics of thermal spallation and use this model to examine existing theories concerning spalling mechanisms. We will report how borehole conditions influence spall production, and discuss implications for macro-scale models of drilling systems.

  10. Liquid lithium target as a high intensity, high energy neutron source

    Science.gov (United States)

    Parkin, Don M.; Dudey, Norman D.

    1976-01-01

    This invention provides a target jet for charged particles. In one embodiment the charged particles are high energy deuterons that bombard the target jet to produce high intensity, high energy neutrons. To this end, deuterons in a vacuum container bombard an endlessly circulating, free-falling, sheet-shaped, copiously flowing, liquid lithium jet that gushes by gravity from a rectangular cross-section vent on the inside of the container means to form a moving web in contact with the inside wall of the vacuum container. The neutrons are produced via break-up of the beam in the target by stripping, spallation and compound nuclear reactions in which the projectiles (deuterons) interact with the target (Li) to produce excited nuclei, which then "boil off" or evaporate a neutron.

  11. Liquid lithium target as a high intensity, high energy neutron source

    International Nuclear Information System (INIS)

    Parkin, D.M.; Dudey, N.D.

    1976-01-01

    The invention described provides a target jet for charged particles. In one embodiment the charged particles are high energy deuterons that bombard the target jet to produce high intensity, high energy neutrons. To this end, deuterons in a vacuum container bombard an endlessly circulating, free-falling, sheet-shaped, copiously flowing, liquid lithium jet that gushes by gravity from a rectangular cross-section vent on the inside of the container means to form a moving web in contact with the inside wall of the vacuum container. The neutrons are produced via break-up of the beam in the target by stripping, spallation and compound nuclear reactions in which the projectiles (deuterons) interact with the target (Li) to produce excited nuclei, which then ''boil off'' or evaporate a neutron

  12. Joint ICTP-IAEA advanced workshop on model codes for spallation reactions

    International Nuclear Information System (INIS)

    Filges, D.; Leray, S.; Yariv, Y.; Mengoni, A.; Stanculescu, A.; Mank, G.

    2008-08-01

    The International Atomic Energy Agency (IAEA) and the Abdus Salam International Centre for Theoretical Physics (ICTP) organised an expert meeting at the ICTP from 4 to 8 February 2008 to discuss model codes for spallation reactions. These nuclear reactions play an important role in a wide domain of applications ranging from neutron sources for condensed matter and material studies, transmutation of nuclear waste and rare isotope production to astrophysics, simulation of detector set-ups in nuclear and particle physics experiments, and radiation protection near accelerators or in space. The simulation tools developed for these domains use nuclear model codes to compute the production yields and characteristics of all the particles and nuclei generated in these reactions. These codes are generally Monte-Carlo implementations of Intra-Nuclear Cascade (INC) or Quantum Molecular Dynamics (QMD) models, followed by de-excitation (principally evaporation/fission) models. Experts have discussed in depth the physics contained within the different models in order to understand their strengths and weaknesses. Such codes need to be validated against experimental data in order to determine their accuracy and reliability with respect to all forms of application. Agreement was reached during the course of the workshop to organise an international benchmark of the different models developed by different groups around the world. The specifications of the benchmark, including the set of selected experimental data to be compared to the models, were also defined during the workshop. The benchmark will be organised under the auspices of the IAEA in 2008, and the first results will be discussed at the next Accelerator Applications Conference (AccApp'09) to be held in Vienna in May 2009. (author)

  13. Spallation-mechanism and characteristics

    International Nuclear Information System (INIS)

    Strugalski, Z.; Strugalska-Gola, E.; Wojciechowski, A.

    1996-01-01

    Mechanism of spallation is revealed experimentally. Spallation is a complicated nuclear reaction initiated by fast hadron in which three stages may be distinguished: a) the first stage in which the target nucleus is locally damaged, it lasts ∼10 -24 +10 -22 s; b) the slow stage which lasts ∼10 -22 +10 -17 s after the collision started, the damaged and excited nucleus uses to emit the black track leaving particles; c) the final stage in which residual target nucleus uses to split into two or more fragments. Quantitative characteristics of each of the stages are presented. 35 refs

  14. Safety techniques in the change of nuclear systems. Radiation protection at spallation neutron sources and transmutation facilities

    International Nuclear Information System (INIS)

    Nuenighoff, Kay

    2009-01-01

    To push the boundary towards higher neutron fluxes concepts based on spallation reactions have been discussed. Here neutrons are produced by bombarding a heavy metal target (e.g. mercury, tungsten, or tantalum) with high energetic protons. Up to now such facilities could not be realised because of the high power particle accelerators needed. Recent developments of the accelerator technology open the possibility of construction and operating proton accelerators in the MW region. This is demonstrated by construction and commissioning of two MW spallation neutron sources, namely SNS (Oak Ridge, Tennessee, USA) with a power of 1.4 MW and J-PARC (Japan) with 1 MW. The realisation of proton accelerators at this power level will open the way towards energy amplifiers, as proposed e.g. by Carlo Rubbia. Such a facility will not only produce electric power. Furthermore longliving radionuclides can be transmutated into shortlived or even stable nuclides by neutron induced nuclear reactions. A mitigation of the problem of nuclear waste disposal. The above discussed developments prove that accelerators are not only constructed for research, moreover application of these technology became state of the art. With the emergence of particle accelerators in the MW region, radiation protection is confronted with new kind of problems to be solved. Especially the higher kinetic energies of the primary beam particles requires modification and expansion of computer programs well known in nuclear engineering. In contrast to nuclear reactors with kinetic energies up to 2-3 MeV, in spallation reaction secondary particles up to the incident energy in the GeV region will be produced. Problems related to radiation protection have to be considered in an energy range three orders of magnitude higher than known from nuclear reactors. In this thesis existing computer codes are compared and validated with data from selected experiments. Questions concerning radiation protection covers a broad range

  15. Nuclear reactions induced by high-energy alpha particles

    Science.gov (United States)

    Shen, B. S. P.

    1974-01-01

    Experimental and theoretical studies of nuclear reactions induced by high energy protons and heavier ions are included. Fundamental data needed in the shielding, dosimetry, and radiobiology of high energy particles produced by accelerators were generated, along with data on cosmic ray interaction with matter. The mechanism of high energy nucleon-nucleus reactions is also examined, especially for light target nuclei of mass number comparable to that of biological tissue.

  16. Technical development of high intensity proton accelerators in Japan Atomic Energy Research Institute (JAERI)

    International Nuclear Information System (INIS)

    Mizumoto, Motoharu

    1995-01-01

    Science and Technology Agency decided 'Options making extra gains of actinides and fission products (OMEGA)' and to promote the related researches. Also in JAERI, the research on the group separation method for separating transuranic elements, strontium and cesium from high level radioactive wastes has been carried out since the beginning of 1970s. Also the concept of the fast reactors using minor actinide mixture fuel is being established, and the accelerator annihilation treatment utilizing the nuclear spallation reaction by high energy protons has been examined. In this report, from the viewpoint of the application of accelerators to atomic energy field, the annihilation treatment method by the nuclear spallation reaction utilizing high intensity proton accelerators, the plan of the various engineering utilization of proton beam, and the development of accelerators in JAERI are described. The way of thinking on the annihilation treatment of radioactive waste, the system using fast neutrons, the way of thinking on the development of high intensity proton accelerator technology, the steps of the development, the research and development for constructing the basic technology accelerator, 2 MeV beam acceleration test, the basic technology accelerator utilization facility and so on are reported. (K.I.)

  17. Future prospects of imaging at spallation neutron sources

    International Nuclear Information System (INIS)

    Strobl, M.

    2009-01-01

    The advent of state-of-the-art spallation neutron sources is a major step forward in efficient neutron production for most neutron scattering techniques. Although they provide lower time-averaged neutron flux than high flux reactor sources, advantage for different instrumental techniques can be derived from the pulsed time structure of the available flux, which can be translated into energy, respectively, wavelength resolution. Conventional neutron imaging on the other hand relies on an intense continuous beam flux and hence falls short in profiting from the new development. Nevertheless, some recently developed novel imaging techniques require and some can benefit from energy resolution. The impact of the emerging spallation sources on different imaging techniques has been investigated, ways to benefit will be identified (where possible) and prospects of future imaging instruments and possible options and layouts at a spallation neutron source will be discussed and outlined.

  18. Present status of spallation target development. JAERI/KEK Joint Project

    International Nuclear Information System (INIS)

    Hino, R.; Kaminaga, M.; Haga, K.

    2001-01-01

    The Japan Atomic Energy Research Institute (JAERI) and the High Energy Accelerator Research Organization (KEK) are promoting a plan to construct a neutron scattering facility under the JAERI/KEK Joint Project. Design and R and D works are being carried out vigorously for realizing the mercury target system consisting of the mercury target, moderators and reflectors working as a spallation neutron source, as well as a remote handling system for exchanging such components which will be highly irradiated. This report introduces an outline of the present status of design and development activities on the spallation target system. (author)

  19. Analysis of the spallation residues and the associated particles in the reaction Fe+p at 1 GeV per nucleon

    International Nuclear Information System (INIS)

    Le Gentil, E.

    2006-09-01

    SPALADIN is a new type of spallation experiment that has been carried out at the GSI accelerator facility (Germany) in order to improve the modelling of the spallation reaction. This experiment is based on the coincidence measurement in inverse kinematics of the spallation residues and the de-excitation fragments. This work presents the analysis of Fe 56 + p reaction at 1 GeV per nucleon. Results on cross-sections and heavy residue velocity spectra are compared to previous data and enabled us to characterize the setup. Most of the element production cross-sections have been obtained with an uncertainty below 10 per cent. In the particular case of helium, its production cross-section has been measured to be σ(1 GeV) = (598 ± 67) mb. The knowledge of this cross-section is important to assess the irradiation damage undergone by the window separating the accelerator from the target. The study of the de-excitation of the pre-fragment shows that the evaporation of light particles (Z ≤ 2) is the main way of de-excitation whatever the collision centrality. However, the de-excitation through the emission of intermediate mass fragments is observed in 5% of the events and most of these events correspond to a very asymmetric binary breaking. The velocity distributions of light residues (with regards to the mass of the projectile) show a significant disagreement with the average velocities predicted by spallation codes. (A.C.)

  20. Nucleus fragmentation induced by a high-energy hadron

    International Nuclear Information System (INIS)

    Zielinski, P.

    1982-10-01

    The author presents a review about the spallation in hadron reactions. Especially he considers proton-proton correlations at low relative momentum, angular distributions of 30-100 MeV protons, emission of fast deuterons, the vanishing of the Coulomb barrier, fission-like processes, the rise of the heavy fragment yield with energy transfer, proton-deuteron breakup reactions, and the backward emission of fast protons. (HSI)

  1. Technical design report of spallation neutron source facility in J-PARC

    International Nuclear Information System (INIS)

    Sakamoto, Shinichi

    2012-02-01

    One of the experimental facilities in Japan Proton Accelerator Research Complex (J-PARC) is the Materials and Life Science Experimental Facility (MLF), where high-intensity neutron beams are used as powerful probes for basic research on materials and life science, as well as research and development in industrial engineering. Neutrons are generated with nuclear spallation reaction by bombarding a mercury target with high-intensity proton beams. The neutrons are slowed down with supercritical hydrogen moderators and then extracted as beams to each experimental apparatus. The principal design of the spallation neutron source is compiled in this comprehensive report. (author)

  2. Thermal features of spallation window targets

    International Nuclear Information System (INIS)

    Martinez-Val, J. M.; Sordo, F.; Leon, P. T.

    2007-01-01

    Subcritical nuclear reactors have been proposed for a number of applications, from energy production to fertile-to-fissile conversion, and to transmutation of long-lived radio nuclei into stable or much shorter-lived nuclei. The main advantage of subcritical reactors is their large reactivity margin for not to attain prompt-supercritical power surges. On the contrary, subcritical reactors present some economic drawbacks and technical complexities that deserve suitable attention in the Research and Development phase. Namely, they need a very intense neutron source in order to keep the neutron flux and the reactor power at the required level. The most intense neutron source seems to be based on the proton-induced (or deuteron-induced) spallation reaction in heavy nuclei targets, which present very demanding thermal features that must be properly limited. Those limits pose upper bounds to the neutron yield of the target. In turn, the limits depend on the features of the impinging particle beam and the material composition and geometry of the target. Although the potential design window for spallation targets is rather wide, the analysis presented in this paper identifies specific topics that must properly be covered in the detailed project of a spallation source, in order to avoid unacceptable temperatures and mechanical stresses in the most critical parts of the source. In this paper, some calculations are reported on solid targets (water cooled or helium cooled) and molten metals targets. It is seen that thermal-hydraulic and mechanical calculations of spallation targets are fundamental elements in the coherent design of this type of very intense neutron sources. This coherence implies the need of a suitable trade-off among the relevant beam parameters (proton energy, total intensity and cross-section shape) and the features of the target (structural materials, coolant characteristics and target geometry). The goal of maximizing the neutron yield has to be checked

  3. Investigating the intra-nuclear cascade process using the reaction 136Xe on deuterium at 500 AMeV

    Directory of Open Access Journals (Sweden)

    Rejmund F.

    2010-10-01

    Full Text Available More than 600 residual nuclei, formed in the spallation of 136Xe projectiles impinging on deuterium at 500 AMeV of incident energy, have been unambiguously identified and their production cross sections have been determined with high accuracy. By comparing these data to others previously measured for the reactions 136Xe  +  p at 1 AGeV and 136Xe  +  p at 500 AMeV we investigated the role that neutrons play in peripheral collisions and to understand the energy dissipation in frontal collisions in spallation reactions.

  4. Spallation RI beam facility and heavy element nuclear chemistry

    Energy Technology Data Exchange (ETDEWEB)

    Nagame, Yuichiro [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

    1997-11-01

    An outline of the spallation RI (Radioactive Ion) beam facility is presented. Neutron-rich nuclides are produced in the reaction of high intensity (10-1000 {mu}A) protons with energy of 1.5 GeV and an uranium carbide target. Produced nuclides are ionized in an isotope separator on-line (ISOL) and accelerated by the JAERI tandem and the booster linac. Current progress and a future project on the development of the RI beam facility are given. Studies of transactinide elements, including the synthesis of superheavy elements, nuclear structure far from stability, and RI-probed material science are planned with RI beams. An outlook of the transactinide nuclear chemistry studies using neutron-rich RI beams is described. (author)

  5. New aspects of high energy heavy-ion transfer reactions

    International Nuclear Information System (INIS)

    Scott, D.K.

    1975-03-01

    New aspects of heavy ion reactions at incident energies in the region of 10 MeV/nucleon are discussed with an emphasis on the peripheral nature of the collisions, which leads to simplicities in the differential cross sections. The distortion of the peripheral distribution through the interference of direct and multistep processes is used to illustrate aspects of high energy reactions unique to heavy ions. The simplicities of the distributions for reactions on lighter nuclei are exploited to give new information about nuclear structure from direct and compound reactions at high energy. (16 figures, 32 references) (U.S.)

  6. Study of particle transport in a high power spallation target for an accelerator-driven transmutation system

    International Nuclear Information System (INIS)

    Shetty, Nikhil Vittal

    2013-01-01

    AGATE is a project envisaged to demonstrate the feasibility of transmutation in a gas (helium) cooled accelerator-driven system using solid spallation target. Development of the spallation target module and assessing its safety aspects are studied in this work. According to the AGATE concept parameters, 600 MeV protons are delivered on to the segmented tungsten spallation target. The Monte Carlo toolkit Geant4 has been used in the simulation of particle transport. Binary cascade is used to simulate intra-nuclear cascades, along with the G4NDL neutron data library for low energy neutrons (<20 MeV).

  7. Study of particle transport in a high power spallation target for an accelerator-driven transmutation system

    Energy Technology Data Exchange (ETDEWEB)

    Shetty, Nikhil Vittal

    2013-01-31

    AGATE is a project envisaged to demonstrate the feasibility of transmutation in a gas (helium) cooled accelerator-driven system using solid spallation target. Development of the spallation target module and assessing its safety aspects are studied in this work. According to the AGATE concept parameters, 600 MeV protons are delivered on to the segmented tungsten spallation target. The Monte Carlo toolkit Geant4 has been used in the simulation of particle transport. Binary cascade is used to simulate intra-nuclear cascades, along with the G4NDL neutron data library for low energy neutrons (<20 MeV).

  8. Estimation of thermochemical behavior of spallation products in mercury target

    International Nuclear Information System (INIS)

    Kobayashi, Kaoru; Kaminaga, Masanori; Haga, Katsuhiro; Kinoshita, Hidetaka; Aso, Tomokazu; Teshigawara, Makoto; Hino, Ryutaro

    2002-02-01

    In order to examine the radiation safety of a spallation mercury target system, especially source term evaluation, it is necessary to clarify the chemical forms of spallation products generated by spallation reaction with proton beam. As for the chemical forms of spallation products in mercury that involves large amounts of spallation products, these forms were estimated by using the binary phase diagrams and the thermochemical equilibrium calculation based on the amounts of spallation product. Calculation results showed that the mercury would dissolve Al, As, B, Be, Bi, C, Co, Cr, Fe, Ga, Ge, Ir, Mo, Nb, Os, Re, Ru, Sb, Si, Ta, Tc, V and W in the element state, and Ag, Au, Ba, Br, Ca, Cd, Ce, Cl, Cs, Cu, Dy, Er, Eu, F, Gd, Hf, Ho, I, In, K, La, Li, Lu, Mg, Mn, Na, Nd, Ni, O, Pb, Pd, Pr, Pt, Rb, Rh, S, Sc, Se, Sm, Sn, Sr, Tb, Te, Ti, Tl, Tm, Y, Yb, Zn and Zr in the form of inorganic mercury compounds. As for As, Be, Co, Cr, Fe, Ge, Ir, Mo, Nb, Os, Pt, Re, Ru, Se, Ta, V, W and Zr, precipitation could be occurred when increasing the amounts of spallation products with operation time of the spallation target system. On the other hand, beryllium-7 (Be-7), which is produced by spallation reaction of oxygen in the cooling water of a safety hull, becomes the main factor of the external exposure to maintain the cooling loop. Based on the thermochemical equilibrium calculation to Be-H 2 O binary system, the chemical forms of Be in the cooling water were estimated. Then the Be could exist in the form of cations such as BeOH + , BeO + and Be 2+ under the condition of less than 10 -8 of the Be mole fraction in the cooling water. (author)

  9. Neutron-induced transmutation reactions in Np-237, Pu-238, and Pu-239 at the massive natural uranium spallation target

    Czech Academy of Sciences Publication Activity Database

    Závorka, L.; Adam, Jindřich; Baldin, A. A.; Čaloun, Pavel; Chilap, V. V.; Furman, W.; Kadykov, M. G.; Khushvaktov, J.; Pronskikh, V. S.; Solnyshkin, A. A.; Sotnikov, V.; Stegailov, V. I.; Suchopár, Martin; Tsoupko-Sitnikov, V. M.; Tyutyunnikov, S. I.; Voronko, V.; Vrzalová, Jitka

    2015-01-01

    Roč. 349, APR (2015), s. 31-38 ISSN 0168-583X R&D Projects: GA MŠk LG14004 Institutional support: RVO:61389005 Keywords : ADS * spent nuclear fuel * transmutation reaction * spallation neutrons Subject RIV: BG - Nuclear , Atomic and Molecular Physics, Colliders Impact factor: 1.389, year: 2015

  10. Neutronics of pulsed spallation neutron sources

    CERN Document Server

    Watanabe, N

    2003-01-01

    Various topics and issues on the neutronics of pulsed spallation neutron sources, mainly for neutron scattering experiments, are reviewed to give a wide circle of readers a better understanding of these sources in order to achieve a high neutronic performance. Starting from what neutrons are needed, what the spallation reaction is and how to produce slow-neutrons more efficiently, the outline of the target and moderator neutronics are explained. Various efforts with some new concepts or ideas have already been devoted to obtaining the highest possible slow-neutron intensity with desired pulse characteristics. This paper also reviews the recent progress of such efforts, mainly focused on moderator neutronics, since moderators are the final devices of a neutron source, which determine the source performance. Various governing parameters for neutron-pulse characteristics such as material issues, geometrical parameters (shape and dimensions), the target-moderator coupling scheme, the ortho-para-hydrogen ratio, po...

  11. Workshop: Research and development plans for high power spallation neutron testing at BNL

    International Nuclear Information System (INIS)

    1996-01-01

    This report consists of vugraphs from presentations at the meeting. The papers covered the following topics: (1) APS as a proton source; (2) target status for NSNS (National Spallation Neutron Source); (3) spallation neutron source in Japan; (4) liquid LiBi flow loop; and (5) research and development plans for high power tests at the AGS

  12. Linac-driven spallation-neutron source

    International Nuclear Information System (INIS)

    Jason, A.J.

    1995-01-01

    Strong interest has arisen in accelerator-driven spallation-neutron sources that surpass existing facilities (such as ISIS at Rutherford or LANSCE at Los Alamos) by more than an order of magnitude in beam power delivered to the spallation target. The approach chosen by Los Alamos (as well as the European Spallation Source) provides the full beam energy by acceleration in a linac as opposed to primary acceleration in a synchrotron or other circular device. Two modes of neutron production are visualized for the source. A short-pulse mode produces 1 MW of beam power (at 60 pps) in pulses, of length less than 1 ms, by compression of the linac macropulse through multi-turn injection in an accumulator ring. A long-pulse mode produces a similar beam power with 1-ms-long pulses directly applied to a target. This latter mode rivals the performance of existing reactor facilities to very low neutron energies. Combination with the short-pulse mode addresses virtually all applications

  13. Low-energy beam transport studies supporting the spallation neutron source 1-MW beam operation.

    Science.gov (United States)

    Han, B X; Kalvas, T; Tarvainen, O; Welton, R F; Murray, S N; Pennisi, T R; Santana, M; Stockli, M P

    2012-02-01

    The H(-) injector consisting of a cesium enhanced RF-driven ion source and a 2-lens electrostatic low-energy beam transport (LEBT) system supports the spallation neutron source 1 MW beam operation with ∼38 mA beam current in the linac at 60 Hz with a pulse length of up to ∼1.0 ms. In this work, two important issues associated with the low-energy beam transport are discussed: (1) inconsistent dependence of the post-radio frequency quadrupole accelerator beam current on the ion source tilt angle and (2) high power beam losses on the LEBT electrodes under some off-nominal conditions compromising their reliability.

  14. Spallation production of neutron deficient radioisotopes in North America

    International Nuclear Information System (INIS)

    Jamriska, D.J.; Peterson, E.J.; Carty, J.

    1997-01-01

    The US Department of Energy produces a number of neutron deficient radioisotopes by high energy proton induced spallation reactions in accelerators at Los Alamos National Laboratory in New Mexico and Brookhaven National Laboratory in New York. Research isotopes are also recovered from targets irradiated at TRIUMF in British Columbia, Canada. The radioisotopes recovered are distributed for use in nuclear medicine, environmental research, physics research, and industry worldwide. In addition to the main product line of Sr-82 from either Mo or Rb targets, Cu-67 from ZnO targets, and Ge-68 and RbBr targets, these irradiation facilities also produce some unique isotopes in quantities not available from any other source such as Al-26, Mg-28, Si-32, Ti-44, Fe-52, Gd-148, and Hg-194. The authors will describe the accelerator irradiation facilities at the Los Alamos and Brookhaven National Laboratories. The high level radiochemical processing facilities at Los Alamos and brief chemical processes will be described

  15. Quasielastic high-resolution time-of-flight spectrometers employing multi-disk chopper cascades for spallation sources

    International Nuclear Information System (INIS)

    Lechner, R.E.

    2001-01-01

    The design of multi-disk chopper time-of-flight (MTOF) spectrometers for high-resolution quasielastic and low-energy inelastic neutron scattering at spallation sources is discussed in some detail. A continuously variable energy resolution (1 μeV to 10 meV), and a large dynamic range (1 μeV to 100 meV), are outstanding features of this type of instrument, which are easily achieved also at a pulsed source using state-of-the-art technology. The method of intensity-resolution optimization of MTOF spectrometers at spallation sources is treated on the basis of the requirement of using (almost) 'all the neutrons of the pulse', taking into account the constant, but wavelength-dependent duration of the source pulse. It follows, that the optimization procedure (which is slightly different from that employed in the steady-state source case) should give priority to the highest resolution, whenever such a choice becomes necessary. This leads to long monochromator distances (L l2 ) of the order of 50 m, for achieving resolutions now available at reactor sources. A few examples of spectrometer layout and corresponding design parameters for large-angle and for small-angle quasielastic scattering instruments are given. In the latter case higher energy resolution than for large-angle scattering is required and achieved. The use of phase-space transformers, neutron wavelength band-pass filters and multichromatic operation for the purpose of intensity-resolution optimization are discussed. This spectrometer can be designed to make full use of the pulsed source peak flux. Therefore, and because of a number of improvements, high resolution will be available at high intensity: for any given resolution the total intensity at the detectors, when placed at one of the planned new spallation sources (SNS, JSNS, ESS, AUSTRON) will be larger by at least three orders of magnitude than the total intensity of any of the presently existing instruments of this type in routine operation at steady

  16. Application of on-line HPLC-ICP-MS for the determination of the nuclide abundances of lanthanides produced via spallation reactions in an irradiated tantalum target of a spallation neutron source

    International Nuclear Information System (INIS)

    Kerl, W.; Becker, J.S.; Dietze, H.J.

    1998-01-01

    An analytical procedure has been developed for the determination of spallation nuclides in an irradiated tantalum target using HPLC coupled on-line to ICP-MS after dissolution and separation of the tantalum matrix. Pieces of tantalum were taken from different locations of the irradiated tantalum target which had been used as the target material in a spallation neutron source. Tantalum was dissolved in a HNO 3 /HF mixture and the tantalum matrix was separated by liquid-liquid extraction so that only the spallation nuclides were left in the sample solutions. The major fraction of the spallation nuclides in the tantalum target are lanthanide metals in the μg g -1 concentration range determined in the present study. Additional reaction products are formed by the irradiation of trace impurities in the original tantalum target. The nuclide abundances of the lanthanide metals measured in the tantalum target differ significantly from the natural isotopic composition so that a lot of isobaric interferences of long-lived radionuclides and stable isotopes in the mass spectrum are to be expected. Therefore, all the lanthanide metals had to be separated chemically prior to their mass spectrometric determination. The separation of all rare earth elements was performed by ion chromatography on-line to ICP-MS. The nuclide abundances of each lanthanide were determined using a sensitive double-focusing sector field inductively coupled plasma mass spectrometer. The nuclide abundances of the lanthanides in the irradiated tantalum target calculated theoretically and the experimental results obtained by on-line HPLC-ICP-MS proved to be in good agreement. (orig.)

  17. Measurement of isotopic cross sections of spallation residues in 800 A MeV {sup 197}Au + p collisions

    Energy Technology Data Exchange (ETDEWEB)

    Rejmund, F.; Mustapha, B.; Bernas, M.; Stephan, C.; Taieb, J.; Tassan-Got, L. [Institut de Physique Nucleaire, (IN2P3/CNRS) 91 - Orsay (France); Armbruster, P.; Benlliure, J.; Enqvist, T.; Schmidt, K.H.; Taieb, J. [GSI, Planckstrasse, Darmstadt (Germany); Benlliure, J. [Universidad de Santiago de Compostela (Spain); Boudard, A.; Legrain, R.; Leray, S.; Volant, C. [CEA/Saclay, Dept. d' Astrophysique, de la Physique des Particules, de la Physique Nucleaire et de l' Instrumentation Associee (DAPNIA), 91 - Gif-sur-Yvette (France); Dufour, J.P. [CENBG, IN2P3, 33 - Gradignan (France)

    2000-07-01

    The spallation of {sup 197}Au by 800 MeV protons was investigated in inverse kinematics at GSI, Darmstadt, by use of a {sup 197}Au beam bombarding a liquid-hydrogen target. The fragment separator (FRS) was used to select and identify the reaction products prior to {beta} decay. The individual production cross sections and the kinematical properties of 396 isotopes for all elements between mercury (Z=80) and neodymium (Z=60) have been measured. A comparison with Monte Carlo calculations based on different two-step models of the spallation reaction is given. The shape of the isotopic distributions close to the projectile is found to differ strongly from that resulting from aluminium-induced fragmentation of {sup 197}Au. The mean kinetic energies of the fragments are deduced from the experimental data. The importance of the new data to improve our understanding of the spallation mechanism and the relevance for the design of accelerator-driven sub-critical reactors is discussed. (authors)

  18. An attempt to analyse spallation yelds with a four-parameter formula

    International Nuclear Information System (INIS)

    Martins, J.B.; Napoli, V. di; Tavares, O.A.P.; Terranova, M.L.; Portanova, R.

    1978-09-01

    A semiempirical four-parameter formula, following the formalism of Gupta, is proposed in order to systematise spallation yields. A preliminary test made by comparing calculated and experimentally determined cross sections for 2-GeV bremsstrahlung-induced spallation in natural copper gave very encouraging results (a coefficient of reproducibility R = 1.7 or better). The formula will be used for an exhaustive study of intermediate- and high-energy photospallation of medium-weight nuclei [pt

  19. Analysis for fragmentation products of proton-induced reactions on Pb with energy up to GeV

    International Nuclear Information System (INIS)

    Fan Sheng; Li Zhuxia; Zhao Zhixiang; Ding Dazhao

    2002-01-01

    The mass and charge distribution of residual products produced in the spallation reaction needs to be studied because it can provide useful information for the disposal of nuclear and the radiation damage in the spallation target. The mass and charge distribution of the spallation products is studied by using quantum molecular dynamic (QMD) models. The simulation results are well agreed with the experimental data of the spallation fragment and empirical formula. However, QMD model does not include the fission process; the calculations can not reproduce the fission fragment. The fission model is introduced into QMD model to investigate the fragment products from proton-induced reactions on Pb. The results are in good agreement with the experimental data

  20. Estimation of thermochemical behavior of spallation products in mercury target

    Energy Technology Data Exchange (ETDEWEB)

    Kobayashi, Kaoru; Kaminaga, Masanori; Haga, Katsuhiro; Kinoshita, Hidetaka; Aso, Tomokazu; Teshigawara, Makoto; Hino, Ryutaro [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

    2002-02-01

    In order to examine the radiation safety of a spallation mercury target system, especially source term evaluation, it is necessary to clarify the chemical forms of spallation products generated by spallation reaction with proton beam. As for the chemical forms of spallation products in mercury that involves large amounts of spallation products, these forms were estimated by using the binary phase diagrams and the thermochemical equilibrium calculation based on the amounts of spallation product. Calculation results showed that the mercury would dissolve Al, As, B, Be, Bi, C, Co, Cr, Fe, Ga, Ge, Ir, Mo, Nb, Os, Re, Ru, Sb, Si, Ta, Tc, V and W in the element state, and Ag, Au, Ba, Br, Ca, Cd, Ce, Cl, Cs, Cu, Dy, Er, Eu, F, Gd, Hf, Ho, I, In, K, La, Li, Lu, Mg, Mn, Na, Nd, Ni, O, Pb, Pd, Pr, Pt, Rb, Rh, S, Sc, Se, Sm, Sn, Sr, Tb, Te, Ti, Tl, Tm, Y, Yb, Zn and Zr in the form of inorganic mercury compounds. As for As, Be, Co, Cr, Fe, Ge, Ir, Mo, Nb, Os, Pt, Re, Ru, Se, Ta, V, W and Zr, precipitation could be occurred when increasing the amounts of spallation products with operation time of the spallation target system. On the other hand, beryllium-7 (Be-7), which is produced by spallation reaction of oxygen in the cooling water of a safety hull, becomes the main factor of the external exposure to maintain the cooling loop. Based on the thermochemical equilibrium calculation to Be-H{sub 2}O binary system, the chemical forms of Be in the cooling water were estimated. Then the Be could exist in the form of cations such as BeOH{sup +}, BeO{sup +} and Be{sup 2+} under the condition of less than 10{sup -8} of the Be mole fraction in the cooling water. (author)

  1. Investigation of mechanisms of production of argon, krypton and xenon isotopes formed in heavy targets by protons with an energy ranging from 0.15 to 24 GeV

    International Nuclear Information System (INIS)

    Sauvageon, Henri

    1981-01-01

    As experimental results of the investigation of interactions between high-energy protons and nucleus generally lead to the distinction between four types of reaction mechanisms (spallation, fission, fragmentation and isotope production), this research thesis reports the study of this mechanisms by using the so-called 'thick target - thick collector' experiment and by studying the production of various isotopes of rare gases (argon, krypton, xenon). These isotopes are produced by using platinum, gold, bismuth and thorium targets bombarded by protons with an energy ranging from 0.15 to 24 GeV. The author presents the experimental methods (target preparation and irradiation, rare gas analysis system), reports the analysis of thick target - thick-collector experiments (vector-based representation, path determination, path-curve energy, corrections of experimental data, excitation energy of the intermediate nucleus), presents the experimental results, and discusses their interpretation (two-stage model of high energy nuclear reactions, isotopes produced by spallation and by fission, isotopes produced by deep spallation, representations of mechanisms of fragmentation and deep spallation)

  2. Simulation of a high energy neutron irradiation facility at beamline 11 of the China Spallation Neutron Source

    Energy Technology Data Exchange (ETDEWEB)

    Tairan, Liang [School of Physics and Electronic Information Inner Mongolia University for the Nationalities, Tongliao 028043 (China); Zhiduo, Li [Dongguan Branch, Institute of High Energy Physics, CAS, Beijing 100049 (China); Wen, Yin, E-mail: wenyin@aphy.iphy.ac.cn [Dongguan Branch, Institute of High Energy Physics, CAS, Beijing 100049 (China); Institute of Physics, CAS, P.O. Box 603, Beijing 100190 (China); Fei, Shen [Dongguan Branch, Institute of High Energy Physics, CAS, Beijing 100049 (China); Quanzhi, Yu [Dongguan Branch, Institute of High Energy Physics, CAS, Beijing 100049 (China); Institute of Physics, CAS, P.O. Box 603, Beijing 100190 (China); Tianjiao, Liang [Dongguan Branch, Institute of High Energy Physics, CAS, Beijing 100049 (China)

    2017-07-11

    The China Spallation Neutron Source (CSNS) will accommodate 20 neutron beamlines at its first target station. These beamlines serve different purposes, and beamline 11 is designed to analyze the degraded models and damage mechanisms, such as Single Event Effects in electronic components and devices for aerospace electronic systems. This paper gives a preliminary discussion on the scheme of a high energy neutron irradiation experiment at the beamline 11 shutter based on the Monte Carlo simulation method. The neutron source term is generated by calculating the neutrons scattering into beamline 11 with a model that includes the target-moderator-reflector area. Then, the neutron spectrum at the sample position is obtained. The intensity of neutrons with energy of hundreds of MeV is approximately 1E8 neutron/cm{sup 2}/s, which is useful for experiments. The displacement production rate and gas productions are calculated for common materials such as tungsten, tantalum and SS316. The results indicate that the experiment can provide irradiation dose rate ranges from 1E-5 to 1E-4 dpa per operating year. The residual radioactivity is also calculated for regular maintenance work. These results give the basic reference for the experimental design.

  3. Thin and thick target benchmark investigations to validate spallation physics models

    International Nuclear Information System (INIS)

    Filges, D.; Neef, R.D.; Goldenbaum, F.; Nuenighoff, K.; Galin, J.; Letourneau, A.; Lott, B.; Patois, Y.; Schroeder, W.N.

    1999-01-01

    In the ESS (European Spallation Source) study report several areas have been identified where further spallation physics research and code validation is urgently needed: Neutron and charged particle production and multiplicities above one GeV incident protons, energy deposition and heating, material damage parameters, radioactivity and after heat, and high energy source shielding. All simulation calculations will be done using the Juelich HERMES code system. For this purpose various collaborations were organised. One of the collaborations is NESSI (Neutron Scintillator Silicon Detector), which concerns fundamental data as cross-section measurements on neutron multiplicities and charged particles for different ESS relevant materials. (author)

  4. Predicting Induced Radioactivity at High Energy Accelerators

    Energy Technology Data Exchange (ETDEWEB)

    Fasso, Alberto

    1999-08-27

    Radioactive nuclides are produced at high-energy electron accelerators by different kinds of particle interactions with accelerator components and shielding structures. Radioactivity can also be induced in air, cooling fluids, soil and groundwater. The physical reactions involved include spallations due to the hadronic component of electromagnetic showers, photonuclear reactions by intermediate energy photons and low-energy neutron capture. Although the amount of induced radioactivity is less important than that of proton accelerators by about two orders of magnitude, reliable methods to predict induced radioactivity distributions are essential in order to assess the environmental impact of a facility and to plan its decommissioning. Conventional techniques used so far are reviewed, and a new integrated approach is presented, based on an extension of methods used at proton accelerators and on the unique capability of the FLUKA Monte Carlo code to handle the whole joint electromagnetic and hadronic cascade, scoring residual nuclei produced by all relevant particles. The radiation aspects related to the operation of superconducting RF cavities are also addressed.

  5. Reaction mechanism in high energy heavy-ion collisions

    International Nuclear Information System (INIS)

    Tanihata, Isao.

    1982-04-01

    The reaction mechanism in high energy heavy-ion collision is discussed. The discussion is mainly based on the experimental data. Empirical equations have been given for the total cross-sections of nucleus-nucleus reactions and the reaction cross-sections. These cross-sections are well described by the geometrical size of the colliding nuclei. The cross-sections are also understood by microscopic calculation. The charged particle multiplicity gives additional information about the geometrical aspect of heavy ion collision. The data suggested that the total energy, independent of projectile size, is most important for determining the multiplicity. The inclusive proton spectrum in a heavy ion collision showed two distinct regions. The one is the fragment region, and the other the participant region. The spectral shapes of inclusive pion spectra are reasonably well explained by the Coulomb interaction of pions with nuclear fragments. The high energy heavy ion reaction occurs in the overlap region of the projectile and target. This has been tested by measuring the number of participants for various reactions. The space and the time structure of the collision are also discussed in this paper as well as the dynamical aspects of the collision. (Kato, T.)

  6. Materials for spallation neutron sources

    International Nuclear Information System (INIS)

    Sommer, W.F.; Daemen, L.L.

    1996-03-01

    The Workshop on Materials for Spallation Neutron Sources at the Los Alamos Neutron Science Center, February 6 to 10, 1995, gathered scientists from Department of Energy national laboratories, other federal institutions, universities, and industry to discuss areas in which work is needed, successful designs and use of materials, and opportunities for further studies. During the first day of the workshop, speakers presented overviews of current spallation neutron sources. During the next 3 days, seven panels allowed speakers to present information on a variety of topics ranging from experimental and theoretical considerations on radiation damage to materials safety issues. An attempt was made to identify specific problems that require attention within the context of spallation neutron sources. This proceedings is a collection of summaries from the overview sessions and the panel presentations

  7. High energy photons production in nuclear reactions

    International Nuclear Information System (INIS)

    Nifenecker, H.; Pinston, J.A.

    1990-01-01

    Hard photon production, in nucleus-nucleus collisions, were studied at beam energies between 10 and 125 MeV. The main characteristics of the photon emission are deduced. They suggest that the neutron-proton collisions in the early stage of the reaction are the main source of high energy gamma-rays. An overview of the theoretical approaches is given and compared with experimental results. Theoretical attempts to include the contribution of charged pion exchange currents to photon production, in calculations of proton-nucleus-gamma and nucleus-nucleus-gamma reactions, showed suitable fitting with experimental data

  8. Materials performance experience at spallation neutron sources

    Energy Technology Data Exchange (ETDEWEB)

    Sommer, W.F. [Los Alamos National Laboratory, NM (United States)

    1995-10-01

    There is a growing, but not yet substantial, data base for materials performance at spallation neutron sources. Specially designed experiments using medium energy protons (650 MeV) have been conducted at the Proton Irradiation Experiment (PIREX) facility at the Swiss Nuclear Institute accelerator (SIN). Specially designed experiments using 760-800 MeV copper target have been completed at the Los Alamos Spallation Radiation Effects Facility (LASREF) at Los Alamos Meson Physics Facility (LAMPF). An extensive material testing program was initiated at LASREF in support of the German spallation neutron source (SNQ) project, before it terminated in 1985.

  9. Neutronic Design Calculations on Moderators for the Spallation Neutron Source (SNS)

    International Nuclear Information System (INIS)

    Murphy, D.B.

    1999-01-01

    The Spallation Neutron Source (SNS) to be built at the Oak Ridge National Laboratory will provide an intense source of neutrons for a large variety of experiments. It consists of a high-energy (1-GeV) and high-power (∼1-MW) proton accelerator, an accumulator ring, together with a target station and an experimental area. In the target itself, the proton beam will produce neutrons via the spallation process and these will be converted to low-energy ( 2 O moderators. Extensive engineering design work has been conducted on the moderator vessels. For our studies we have produced realistic neutronic representations of these moderators. We report on neutronic studies conducted on these representations of the moderators using Monte Carlo simulation techniques

  10. Spallation source neutron target systems

    International Nuclear Information System (INIS)

    Russell, G.; Brown, R.; Collier, M.; Donahue, J.

    1996-01-01

    This is the final report for a two-year, Laboratory-Directed Research and Development (LDRD) project at the Los Alamos National Laboratory (LANL). The project sought to design a next-generation spallation source neutron target system for the Manuel Lujan, Jr., Neutron Scattering Center (LANSCE) at Los Alamos. It has been recognized for some time that new advanced neutron sources are needed in the US if the country is to maintain a competitive position in several important scientific and technological areas. A recent DOE panel concluded that the proposed Advanced Neutron Source (a nuclear reactor at Oak Ridge National Laboratory) and a high-power pulsed spallation source are both needed in the near future. One of the most technically challenging designs for a spallation source is the target station itself and, more specifically, the target-moderator-reflector arrangement. Los Alamos has demonstrated capabilities in designing, building, and operating high-power spallation-neutron-source target stations. Most of the new design ideas proposed worldwide for target system design for the next generation pulsed spallation source have either been conceived and implemented at LANSCE or proposed by LANSCE target system designers. These concepts include split targets, flux-trap moderators, back scattering and composite moderators, and composite reflectors

  11. Neutron Production in Spallation Reactions of 0.9 and 1.5 GeV Protons on a Thick Lead Target. Comparison between Experimental Data and Monte-Carlo Simulations

    CERN Document Server

    Krasa, A; Bradnova, V; Caloun, P; Chultem, D; Henzl, V; Henzlová, D; Kalinnikov, V G; Krivopustov, M I; Krízek, F; Kugler, A; Majerle, M; Solnyshkin, A A; Stegailov, V I; Tsoupko-Sitnikov, V M; Tumendelger, T; Vasilev, S I; Wagner, V; Nuclear Physics Institute of Academy of Sciences of Czech Republic, Rez, Czech Republic

    2005-01-01

    This paper reports on two experiments performed at the Synchrophasotron/Nuclotron accelerator complex at JINR. Relativistic protons with energies 885 MeV and 1.5 GeV hit a massive cylindrical lead target. The spatial and energetic distributions of the neutron field produced by the spallation reactions were measured by the activation of Al, Au, Bi, Co, and Cu foils placed on the surface of the target and close to it. The yields of the radioactive nuclei produced by threshold reactions in these foils were determined by the analyses of their $\\gamma$ spectra. The comparison with Monte-Carlo based simulations was performed both with the LAHET+MCNP code and the MCNPX code.

  12. Neutron production in spallation reactions of 0.9 and 1.5 GeV protons on a thick lead target. Comparison between experimental data and Monte-Carlo simulations

    International Nuclear Information System (INIS)

    Krasa, A.; Krizek, F.; Wagner, V.; Kugler, A.; Henzl, V.; Henzlova, D.; Majerle, M.; Adam, J.; Caloun, P.; Bradnova, V.; Chultem, D.; Kalinnikov, V.G.; Krivopustov, M.I.; Solnyshkin, A.A.; Stegajlov, V.I.; Tsupko-Sitnikov, V.M.; Tumehndehlgehr, Ts.; Vasil'ev, S.I.

    2005-01-01

    This paper reports on two experiments performed at the Synchrophasotron/Nuclotron accelerator complex at JINR. Relativistic protons with energies 885 MeV and 1.5 GeV hit a massive cylindrical lead target. The spatial and energetic distributions of the neutron field produced by the spallation reactions were measured by the activation of Al, Au, Bi, Co, and Cu foils placed on the surface of the target and close to it. The yields of the radioactive nuclei produced by threshold reactions in these foils were determined by the analyses of their γ spectra. The comparison with Monte-Carlo based simulations was performed both with the LAHET+MCNP code and the MCNPX code

  13. Spallation neutron production and the current intra-nuclear cascade and transport codes

    International Nuclear Information System (INIS)

    Filges, D.; Goldenbaum, F.

    2001-01-01

    A recent renascent interest in energetic proton-induced production of neutrons originates largely from the inception of projects for target stations of intense spallation neutron sources, like the planned European Spallation Source (ESS), accelerator-driven nuclear reactors, nuclear waste transmutation, and also from the application for radioactive beams. In the framework of such a neutron production, of major importance is the search for ways for the most efficient conversion of the primary beam energy into neutron production. Although the issue has been quite successfully addressed experimentally by varying the incident proton energy for various target materials and by covering a huge collection of different target geometries --providing an exhaustive matrix of benchmark data-- the ultimate challenge is to increase the predictive power of transport codes currently on the market. To scrutinize these codes, calculations of reaction cross-sections, hadronic interaction lengths, average neutron multiplicities, neutron multiplicity and energy distributions, and the development of hadronic showers are confronted with recent experimental data of the NESSI collaboration. Program packages like HERMES, LCS or MCNPX master the prevision of reaction cross-sections, hadronic interaction lengths, averaged neutron multiplicities and neutron multiplicity distributions in thick and thin targets for a wide spectrum of incident proton energies, geometrical shapes and materials of the target generally within less than 10% deviation, while production cross-section measurements for light charged particles on thin targets point out that appreciable distinctions exist within these models. (orig.)

  14. Spallation neutron production and the current intra-nuclear cascade and transport codes

    Science.gov (United States)

    Filges, D.; Goldenbaum, F.; Enke, M.; Galin, J.; Herbach, C.-M.; Hilscher, D.; Jahnke, U.; Letourneau, A.; Lott, B.; Neef, R.-D.; Nünighoff, K.; Paul, N.; Péghaire, A.; Pienkowski, L.; Schaal, H.; Schröder, U.; Sterzenbach, G.; Tietze, A.; Tishchenko, V.; Toke, J.; Wohlmuther, M.

    A recent renascent interest in energetic proton-induced production of neutrons originates largely from the inception of projects for target stations of intense spallation neutron sources, like the planned European Spallation Source (ESS), accelerator-driven nuclear reactors, nuclear waste transmutation, and also from the application for radioactive beams. In the framework of such a neutron production, of major importance is the search for ways for the most efficient conversion of the primary beam energy into neutron production. Although the issue has been quite successfully addressed experimentally by varying the incident proton energy for various target materials and by covering a huge collection of different target geometries --providing an exhaustive matrix of benchmark data-- the ultimate challenge is to increase the predictive power of transport codes currently on the market. To scrutinize these codes, calculations of reaction cross-sections, hadronic interaction lengths, average neutron multiplicities, neutron multiplicity and energy distributions, and the development of hadronic showers are confronted with recent experimental data of the NESSI collaboration. Program packages like HERMES, LCS or MCNPX master the prevision of reaction cross-sections, hadronic interaction lengths, averaged neutron multiplicities and neutron multiplicity distributions in thick and thin targets for a wide spectrum of incident proton energies, geometrical shapes and materials of the target generally within less than 10% deviation, while production cross-section measurements for light charged particles on thin targets point out that appreciable distinctions exist within these models.

  15. The biological shield of a high-intensity spallation source: a monte Carlo design study

    International Nuclear Information System (INIS)

    Koprivnikar, I.; Schachinger, E.

    2004-01-01

    The design of high-intensity spallation sources requires the best possible estimates for the biological shield. The applicability of three-dimensional Monte Carlo simulation in the design of the biological shield of a spallation source will be discussed. In order to achieve reasonable computing times along with acceptable accuracy, biasing techniques are to be employed and it was the main purpose of this work to develop a strategy for an effective Monte Carlo simulation in shielding design. The most prominent MC computer codes, namely MCNPX and FLUKA99, have been applied to the same model spallation source (the European Spallation Source) and on the basis of the derived strategies, the design and characteristics of the target station shield are discussed. It is also the purpose of the paper to demonstrate the application of the developed strategy for the design of beam lines with their shielding using as an example the target-moderator-reflector complex of the ESS as the primary particle source. (author)

  16. Target designs for the Brookhaven National Laboratory 5-MW pulsed spallation neutron source

    International Nuclear Information System (INIS)

    Ludewig, H.; Todosow, M.; Powell, J.R.

    1996-01-01

    A feasibility study of a compact high power density target for a spallation neutron source was under-taken. The target arrangement consists primarily of heavy metal, with appropriate cooling passages. A high intensity proton beam of intermediate energy is directed at the target, where it interacts with the heavy metal nuclei. The subsequent spallation reactions produce several neutrons per proton resulting in an intense neutron source. The proton beam is assumed to havean energy of 5 MW, and to be cyclic with a repetition rate of 10Hz and 50Hz. The study was divided into two broad sections. First, an analysis of preliminary target designs was undertaken to ensure the overall feasibility of the concepts involved in the design and eventual construction of such a high power density target. Second, two proposed target designs, based on the first set of analyses, are investigated in more detail. Special care is taken to ensure that the neutron fluxes in the moderator are at the desired level no material compatibility problems exist,and the target is able to operate in a reliable and safe manner. Several target materials, coolant types, and target arrangements are investigated in the first section. The second section concentrates on a single target material and geometric arrangement. However, several structural material choices continue to be investigated with the aim of minimizing the effects of structural heating, and associated thermally induced stresses. In the final section the conclusions of this preliminary study are summarized

  17. Design of the MYRRHA Spallation Target Assembly

    International Nuclear Information System (INIS)

    Keijers, S.; Fernandez, R.; Stankovskiy, A.; Kennedy, G.; Van Tichelen, K.

    2015-01-01

    MYRRHA (Multi-purpose hybrid Research Reactor for High-tech Applications) is a multi-purpose research facility currently being developed at SCK.CEN. MYRRHA is based on the ADS (Accelerator Driven System) concept where a proton accelerator, a spallation target and a subcritical reactor are coupled. MYRRHA will demonstrate the ADS full concept by coupling these three components at a reasonable power level. As a flexible irradiation facility, the MYRRHA research reactor will be able to work in both critical and subcritical modes. In this way, MYRRHA will allow fuel developments for innovative reactor systems, material research for GEN IV and fusion reactors, and radioisotope production for medical and industrial applications. MYRRHA will be cooled by Lead Bismuth Eutectic (LBE) and will play an important role in the development of the Pb-alloys technology needed for the LFR (Lead Fast Reactor) GEN IV concept. This paper describes the evolution of the MYRRHA spallation target design. In the early phase of the MYRRHA project (XT-ADS), the target design was based on a dedicated spallation loop inside the primary reactor vessel. Within the core, the 3 central fuel assembly positions were occupied by the spallation target, which enabled a windowless design created by a free surface of LBE facing the proton beam. The windowless option was preferred because of high heat loads in combination with severe irradiation damage in the target region would result in unacceptably short lifetimes of a target window. The LBE in the loop served as spallation target and as target coolant, but was separated from the LBE cooling the reactor core. The loop was equipped with its own pump, heat exchanger and conditioning system. The change from cyclotron to linear accelerator allowed the increase in proton energy from 350 MeV to 600 MeV. This modification led to an important reduction of the specific heat load at the target level and an improvement of the neutronic performance. In addition to

  18. Study of spallation residues of gold at 0.8 GeV/N in reverse kinematics

    International Nuclear Information System (INIS)

    Tassan-Got, L.; Mustapha, B.; Rejmund, F.

    2000-01-01

    Spallation residue cross-sections of gold have been measured in reverse kinematics. For the first time isotopic distributions have been obtained for such a heavy nucleus at a level of accuracy of 10 %. When compared to model calculations the results appear to be very sensitive to the distribution of excitation energy in the fast step of the reaction. This allows an insight on the mechanism of the energy and momentum deposition. (authors)

  19. Enhanced emission of high-energy photons perpendicular to the reaction plane in α+Th reactions

    International Nuclear Information System (INIS)

    Tegner, P.; Marianski, B.; Morsch, H.P.; Rogge, M.; Bargholtz, C.; Decowski, P.; Zemlo, L.

    1991-01-01

    High-energy photon and neutron emission has been measured in coincidence with fission fragments in α+ 232 Th reactions at 170 MeV. From measurements parallel and perpendicular to the fission plane, anisotropies relative to the reaction plane were determined. The in-plane/out-of-plane intensity ratio is 0.72(7) for photons with energies above 20 MeV and 11(3) for neutrons at 35 MeV. The result for high-energy photons can be explained by nucleon-nucleon bremsstrahlung if the initial flow of nucleons has a correlation to the reaction plane similar to the one observed for fast neutrons

  20. Caging in high energy reactions

    International Nuclear Information System (INIS)

    Ache, H.J.

    1977-01-01

    The concept of caging high energy reactions is considered. It is noted that there is no easy and unambiguous way, short of a complete and very tedious product and mechanistic analysis, which is feasible only for very few systems, to determine the contribution made by caging. It is emphasized that some products resulting from the hot reaction with a certain substrate may be formed via caging while others are not. In research on the mechanism of caging the results of Roots work on the reactions of hot 18 F with the CF 3 CH 3 system seem to provide evidence for caging, with 18 F being the caged moiety, thus proceeding via a radical--radical recombination mechanism. Their work with H 2 S additive also seems to indicate that scavenging via hydrogen abstraction from H 2 S to form does not interfere with the radical--radical recombination consistent with Bunkers molecular approach to explain the cage effects. In other research a series of observations resulting from stereochemical and combined stereochemical density variation techniques seem to favor a caged-complex. It is clear that a more conclusive answer can only be reached by more systematic studies, utilizing the whole range of nuclear reactions such as (n,2n), (n,γ) and E.C. processes in mechanistically well defined systems to elucidate the effect of variations in the recoil energies, by carrying out studies in different solvents or host substances to assess the effect of the physical parameters, such as molecule size and intermolecular interactions on the escape probability or caging efficiencies

  1. Recent research on nuclear reaction using high-energy proton and neutron

    Energy Technology Data Exchange (ETDEWEB)

    Shibata, Tokushi [Tokyo Univ., Tanashi (Japan). Inst. for Nuclear Study

    1997-11-01

    The presently available high-energy neutron beam facilities are introduced. Then some interesting research on nuclear reaction using high-energy protons are reported such as the intermediate mass fragments emission and neutron spectrum measurements on various targets. As the important research using high-energy neutron, the (p,n) reactions on Mn, Fe, and Ni, the elastic scattering of neutrons, and the shielding experiments are discussed. (author)

  2. Spallation Neutron Spectrum on a Massive Lead/Paraffin Target Irradiated with 1 GeV Protons

    CERN Document Server

    Adam, J; Barashenkov, V S; Brandt, R; Golovatiouk, V M; Kalinnikov, V G; Katovsky, K; Krivopustov, M I; Kumar, V; Kumawat, H; Odoj, R; Pronskikh, V S; Solnyshkin, A A; Stegailov, V I; Tsoupko-Sitnikov, V M; Westmeier, W

    2004-01-01

    The spectra of gamma-ray emitted by decaying residual nuclei, produced by spallation neutrons with (n, xn), (n,xnyp), (n,p), (n,gamma) reactions in activation threshold detectors - namely, ^{209}Bi, ^{197}Au, ^{59}Co, ^{115}In, ^{232}Th, were measured in the Laboratory of Nuclear Problems (LNP), JINR, Dubna, Russia. Spallation neutrons were generated by bombarding a 20 cm long cylindrical lead target, 8 cm in diameter, surrounded by a 6 cm thick layer of paraffin moderator, with a 1 GeV proton beam from the Nuclotron accelerator. Reaction rates and spallation neutron spectrum were measured and compared with CASCADE code calculations.

  3. Experimental Study of the Phenomenology of Spallation Neutrons in a Large Lead Block

    CERN Multimedia

    Galvez Altamirano, J; Lopez, C; Perlado, J M; Perez-Navarro, A

    2002-01-01

    %PS211 %title \\\\ \\\\The purpose of PS211 is to determine how neutrons, produced by spallation inside a large Lead volume are slowed down by undergoing a very large number of scatterings, losing each time a small fraction ($\\sim$ 1\\%) of their kinetic energy. The focus is in determining the probability for a spallation neutron produced at an energy of several MeV or more, to survive capture on Lead resonances and to reach resonance energies of materials to be transmuted, such as 5.6 eV for $^{99}$Tc. This process, of Adiabatic Resonance Crossing, involves a subtle interplay between the capture resonances of the Lead medium and of selected impurities. This phenomenology of spallation neutrons in a large Lead volume, is the physics foundation of the Fast Energy Amplifier proposed by C. Rubbia, and could open up new possibilities in the incineration of long-lived nuclear waste such as Actinides or Fission Fragments (e.g. $^{99}$Tc, $^{129}$I, etc.).\\\\ \\\\334 tons of high purity Lead, installed in t7, are exposed to...

  4. Production of Energetic Light Fragments in Spallation Reactions

    Directory of Open Access Journals (Sweden)

    Mashnik Stepan G.

    2014-03-01

    Full Text Available Different reaction mechanisms contribute to the production of light fragments (LF from nuclear reactions. Available models cannot accurately predict emission of LF from arbitrary reactions. However, the emission of LF is important formany applications, such as cosmic-ray-induced single event upsets, radiation protection, and cancer therapy with proton and heavy-ion beams, to name just a few. The cascade-exciton model (CEM and the Los Alamos version of the quark-gluon string model (LAQGSM, as implemented in the CEM03.03 and LAQGSM03.03 event generators used in the Los Alamos Monte Carlo transport code MCNP6, describe quite well the spectra of fragments with sizes up to 4He across a broad range of target masses and incident energies. However, they do not predict high-energy tails for LF heavier than 4He. The standard versions of CEM and LAQGSM do not account for preequilibrium emission of LF larger than 4He. The aim of our work is to extend the preequilibrium model to include such processes. We do this by including the emission of fragments heavier than 4He at the preequilibrium stage, and using an improved version of the Fermi Break-up model, providing improved agreement with various experimental data.

  5. GEM-based thermal neutron beam monitors for spallation sources

    International Nuclear Information System (INIS)

    Croci, G.; Claps, G.; Caniello, R.; Cazzaniga, C.; Grosso, G.; Murtas, F.; Tardocchi, M.; Vassallo, E.; Gorini, G.; Horstmann, C.; Kampmann, R.; Nowak, G.; Stoermer, M.

    2013-01-01

    The development of new large area and high flux thermal neutron detectors for future neutron spallation sources, like the European Spallation Source (ESS) is motivated by the problem of 3 He shortage. In the framework of the development of ESS, GEM (Gas Electron Multiplier) is one of the detector technologies that are being explored as thermal neutron sensors. A first prototype of GEM-based thermal neutron beam monitor (bGEM) has been built during 2012. The bGEM is a triple GEM gaseous detector equipped with an aluminum cathode coated by 1μm thick B 4 C layer used to convert thermal neutrons to charged particles through the 10 B(n, 7 Li)α nuclear reaction. This paper describes the results obtained by testing a bGEM detector at the ISIS spallation source on the VESUVIO beamline. Beam profiles (FWHM x =31 mm and FWHM y =36 mm), bGEM thermal neutron counting efficiency (≈1%), detector stability (3.45%) and the time-of-flight spectrum of the beam were successfully measured. This prototype represents the first step towards the development of thermal neutrons detectors with efficiency larger than 50% as alternatives to 3 He-based gaseous detectors

  6. Disposal strategy of proton irradiated mercury from high power spallation sources

    International Nuclear Information System (INIS)

    Chiriki, Suresh

    2010-01-01

    Large spallation sources are intended to be constructed in Europe (EURISOL: nuclear physics research facility and ESS: European Spallation Source). These facilities would accumulate more than 20 metric tons of irradiated mercury in the target, which has to be treated as highly radioactive and chemo-toxic waste. Liquid waste cannot be tolerated in European repositories. As part of this work on safety/decommissioning of high-power spallation sources, our investigations were focused mainly to study experimentally and theoretically the solidification of liquid mercury waste (selection of an adequate solid mercury form and of an immobilization matrix, chemical engineering process studies on solidification/stabilization and on encapsulating in a matrix). Based on experimental results and supported by literature Hg-chalcogens (HgS, HgSe) will be more stable in repositories than amalgams. Our irradiation experimental studies on mercury waste revealed that mercury sulfide is a reasonable solid for disposal and shows larger stability in possible accidents with water ingress in a repository. Additionally immobilization of mercury in a cement matrix and polysiloxane matrix were tested. HgS formation from liquid target mercury by a wet process is identified as a suitable formation procedure. These investigations reveal that an almost 99.9% elementary Hg conversion can be achieved and that wet process can be reasonably handled under hot cell conditions. (orig.)

  7. Disposal strategy of proton irradiated mercury from high power spallation sources

    Energy Technology Data Exchange (ETDEWEB)

    Chiriki, Suresh

    2010-07-01

    Large spallation sources are intended to be constructed in Europe (EURISOL: nuclear physics research facility and ESS: European Spallation Source). These facilities would accumulate more than 20 metric tons of irradiated mercury in the target, which has to be treated as highly radioactive and chemo-toxic waste. Liquid waste cannot be tolerated in European repositories. As part of this work on safety/decommissioning of high-power spallation sources, our investigations were focused mainly to study experimentally and theoretically the solidification of liquid mercury waste (selection of an adequate solid mercury form and of an immobilization matrix, chemical engineering process studies on solidification/stabilization and on encapsulating in a matrix). Based on experimental results and supported by literature Hg-chalcogens (HgS, HgSe) will be more stable in repositories than amalgams. Our irradiation experimental studies on mercury waste revealed that mercury sulfide is a reasonable solid for disposal and shows larger stability in possible accidents with water ingress in a repository. Additionally immobilization of mercury in a cement matrix and polysiloxane matrix were tested. HgS formation from liquid target mercury by a wet process is identified as a suitable formation procedure. These investigations reveal that an almost 99.9% elementary Hg conversion can be achieved and that wet process can be reasonably handled under hot cell conditions. (orig.)

  8. Mitigation technologies for damage induced by pressure waves in high-power mercury spallation neutron sources (1). Material surface improvement

    International Nuclear Information System (INIS)

    Naoe, Takashi; Futakawa, Masatoshi; Wakui, Takashi; Kogawa, Hiroyuki; Shoubu, Takahisa; Takeuchi, Hirotsugu; Kawai, Masayoshi

    2008-01-01

    Liquid-mercury target systems for MW-class spallation neutron sources are being developed in the world. Proton beams will be used to induce the spallation reaction. At the moment the proton beam hits the target, pressure waves are generated in the mercury because of the abrupt heat deposition. The pressure waves interact with the target vessel leading to negative pressure that may cause cavitation along the vessel wall. Localized impacts by microjets and/or shock waves that are caused by cavitation bubble collapse impose pitting damage on the vessel wall. Bubble collapse behavior was observed by using a high-speed video camera, as well as simulated numerically. Localized impact due to cavitation bubble collapse was quantitatively estimated through comparison between numerical simulation and experiment. A novel surface treatment technique that consists of carburizing and nitriding processes was developed and the treatment condition was optimized to mitigate the pitting damage due to localized impacts. (author)

  9. Target development for the SINQ high-power neutron spallation source

    International Nuclear Information System (INIS)

    Wagner, Werner

    2002-01-01

    SINQ is a 1 MW class research spallation neutron source, driven by the PSI proton accelerator system. In terms of beam power, it is, by a large margin, the most powerful spallation neutron source currently in operation worldwide. As a consequence, target load levels prevail in SINQ which are beyond the realm of existing experience. Therefore, an extensive materials irradiation program (STIP) is currently underway which will help to select the proper structural material and make dependable life time estimates accounting for the real operating conditions that prevail in the facility. In parallel, both theoretical and experimental work is going on within the MEGAPIE (MEGAwatt Pilot Experiment) project, to develop a liquid lead-bismuth spallation target for a beam power level of 1MW

  10. Safety techniques in the change of nuclear systems. Radiation protection at spallation neutron sources and transmutation facilities; Sicherheitstechnik im Wandel Nuklearer Systeme. Strahlenschutz bei Spallationsneutronenquellen und Transmutationsanlagen

    Energy Technology Data Exchange (ETDEWEB)

    Nuenighoff, Kay

    2009-07-01

    To push the boundary towards higher neutron fluxes concepts based on spallation reactions have been discussed. Here neutrons are produced by bombarding a heavy metal target (e.g. mercury, tungsten, or tantalum) with high energetic protons. Up to now such facilities could not be realised because of the high power particle accelerators needed. Recent developments of the accelerator technology open the possibility of construction and operating proton accelerators in the MW region. This is demonstrated by construction and commissioning of two MW spallation neutron sources, namely SNS (Oak Ridge, Tennessee, USA) with a power of 1.4 MW and J-PARC (Japan) with 1 MW. The realisation of proton accelerators at this power level will open the way towards energy amplifiers, as proposed e.g. by Carlo Rubbia. Such a facility will not only produce electric power. Furthermore longliving radionuclides can be transmutated into shortlived or even stable nuclides by neutron induced nuclear reactions. A mitigation of the problem of nuclear waste disposal. The above discussed developments prove that accelerators are not only constructed for research, moreover application of these technology became state of the art. With the emergence of particle accelerators in the MW region, radiation protection is confronted with new kind of problems to be solved. Especially the higher kinetic energies of the primary beam particles requires modification and expansion of computer programs well known in nuclear engineering. In contrast to nuclear reactors with kinetic energies up to 2-3 MeV, in spallation reaction secondary particles up to the incident energy in the GeV region will be produced. Problems related to radiation protection have to be considered in an energy range three orders of magnitude higher than known from nuclear reactors. In this thesis existing computer codes are compared and validated with data from selected experiments. Questions concerning radiation protection covers a broad range

  11. Emission of high-energy, light particles from intermediate-energy heavy-ion reactions

    International Nuclear Information System (INIS)

    Ball, J.B.; Auble, R.L.

    1982-01-01

    One of the early surprises in examining reaction products from heavy ion reactions at 10 MeV/nucleon and above was the large yield of light particles emitted and the high energies to which the spectra of these particles extended. The interpretation of the origin of the high energy light ions has evolved from a picture of projectile excitation and subsequent evaporation to one of pre-equilibrium (or nonequilibrium) emission. The time scale for particle emission has thus moved from one that occurs following the initial collision to one that occurs at the very early stages of the collision. Research at ORNL on this phenomenon is reviewed

  12. Accelerators for energy

    International Nuclear Information System (INIS)

    Inoue, Makoto

    2000-01-01

    A particle accelerator is a device to consume energy but not to produce it. Then, the titled accelerator seems to mean an accelerator for using devices related to nuclear energy. For an accelerator combined to nuclear fissionable fuel, neutron sources are D-T type, (gamma, n) reaction using electron beam type spallation type, and so forth. At viewpoints of powers of incident beam and formed neutron, a spallation type source using high energy proton is told to be effective but others have some advantages by investigation on easy operability, easy construction, combustion with target, energy and directivity of neutron, and so forth. Here were discussed on an accelerator for research on accelerator driven energy system by dividing its researching steps, and on kind, energy, beam intensity, and so forth of an accelerator suitable for it. And, space electric charge effect at beam propagation direction controlled by beam intensity of cyclotron was also commented. (G.K.)

  13. COSMIC-RAY SPALLATION IN RADIO-QUIET ACTIVE GALACTIC NUCLEI: A CASE STUDY OF NGC 4051

    International Nuclear Information System (INIS)

    Turner, T. J.; Miller, L.

    2010-01-01

    We investigate conditions for and consequences of spallation in radio-quiet Seyfert galaxies. The work is motivated by the recent discovery of significant line emission at 5.44 keV in Suzaku data from NGC 4051. The energy of the new line suggests an identification as Cr I Kα emission; however, the line is much stronger than would be expected from material with cosmic abundances, leading to a suggestion of enhancement owing to nuclear spallation of Fe by low-energy cosmic rays from the active nucleus. We find that the highest abundance enhancements are likely to take place in gas out of the plane of the accretion disk and that timescales for spallation could be as short as a few years. The suggestion of a strong nuclear flux of cosmic rays in a radio-quiet active Seyfert galaxy is of particular interest in light of the recent suggestion from Pierre Auger Observatory data that ultra-high-energy cosmic rays may originate in such sources.

  14. A proposal for a long-pulse spallation source at Los Alamos National Laboratory

    International Nuclear Information System (INIS)

    Pynn, R.; Weinacht, D.

    1995-01-01

    Los Alamos National Laboratory is proposing a new spallation neutron source that will provide the US with an internationally competitive facility for neutron science and technology that can be built in approximately three years for less than $100 million. The establishment of a 1-MW, long-pulse spallation source (LPSS) at the Los Alamos Neutron Science Center (LANSCE) will meet many of the present needs of scientists in the neutron scattering community and provide a significant boost to neutron research in the US. The new facility will support the development of a future, more intense spallation neutron source, that is planned by DOE's Office of Energy Research. Together with the existing short pulse spallation source (SPSS) at the Manual Lujan, Jr. Neutron Scattering Center (MLNSC) at Los Alamos, the new LPSS will provide US scientists with a complementary pair of high-performance neutron sources to rival the world's leading facilities in Europe

  15. A proposal for a long-pulse spallation source at Los Alamos National Laboratory

    Energy Technology Data Exchange (ETDEWEB)

    Pynn, R; Weinacht, D [Los Alamos National Lab., NM (United States)

    1995-11-01

    Los Alamos National Laboratory is proposing a new spallation neutron source that will provide the U.S. with an internationally competitive facility for neutron science and technology that can be built in approximately three years for less than $100 million. The establishment of a 1-MW long-pulse spallation source (LPSS) at the Los Alamos Neutron Science Center (LANSCE) will meet many of the present needs of scientists in the neutron scattering community and provide a significant boost to neutron research in the U.S. The new facility will support the development of a future, more intense spallation neutron source, that is planned by DOE`s Office of Energy Research. Together with the existing short pulse spallation source (SPSS) at the Manual Lujan, Jr. Neutron Scattering Center (MLNSC) at Los Alamos, the new LPSS will provide U.S. scientists with a complementary pair of high-performance neutron sources to rival the world`s leading facilities in Europe. (author) 1 ref.

  16. A proposal for a long-pulse spallation source at Los Alamos National Laboratory

    International Nuclear Information System (INIS)

    Pynn, R.; Weinacht, D.

    1995-01-01

    Los Alamos National Laboratory is proposing a new spallation neutron source that will provide the U.S. with an internationally competitive facility for neutron science and technology that can be built in approximately three years for less than $100 million. The establishment of a 1-MW long-pulse spallation source (LPSS) at the Los Alamos Neutron Science Center (LANSCE) will meet many of the present needs of scientists in the neutron scattering community and provide a significant boost to neutron research in the U.S. The new facility will support the development of a future, more intense spallation neutron source, that is planned by DOE's Office of Energy Research. Together with the existing short pulse spallation source (SPSS) at the Manual Lujan, Jr. Neutron Scattering Center (MLNSC) at Los Alamos, the new LPSS will provide U.S. scientists with a complementary pair of high-performance neutron sources to rival the world's leading facilities in Europe. (author) 1 ref

  17. Future of high intensity accelerators in nuclear energy

    International Nuclear Information System (INIS)

    Schriber, S.O.; Fraser, J.S.; Tunnicliffe, P.R.

    1977-08-01

    A possible application for a high mean current, intermediate-energy proton linear accelerator is the ''electrical breeding'' of fuel for nuclear electrical power stations. The possible role of the spallation breeder in the context of a Canadian nuclear power economy and its relationship to nuclear fuel resources are discussed. The production of fissile material using the spallation process in a target containing actinide elements appears desirable and feasible from engineering and economic considerations. Current development work in Canada and some of the outstanding problems are discussed. (author)

  18. Accelerator system of neutron spallation source for nuclear energy technology development

    International Nuclear Information System (INIS)

    Silakhuddin; Mulyaman, Maman

    2002-01-01

    High intensity proton accelerators are at present and developed for applications in neutron spallation sources. The advantages of this source are better safety factor, easy in controlling and spent fuel free. A study of conceptual design of required accelerator system has been carried out. Considering the required proton beam and feasibility in the development stages, a stepped linac system is an adequate choice for now

  19. Spallation studies at Saturne

    Energy Technology Data Exchange (ETDEWEB)

    Frehaut, J. [Centre d`Etudes de Bruyeres-le-Chatel (France)

    1995-10-01

    SATURNE is a synchrotron accelerator which can deliver particles of momentum P and charge Z up to P/Z = 4 GeV/c. Monokinetic neutron beams of momentum up to 2 GeV/c can be produced. The spallation studies deal with measurements of: (i) differential neutron production cross sections from thin targets, (ii) neutron multiplicity distribution for proton and {sup 3}He induced reactions, and (iii) nuclide production in thin target. Measurements on thick or composite targets are under consideration.

  20. Measurement of the spallation reaction {sup 56}Fe+p in inverse kinematics; Messung der Spallationsreaktion {sup 56}Fe+p in inverser Kinematik

    Energy Technology Data Exchange (ETDEWEB)

    Boehmer, M.

    2006-09-25

    In this work the spallation reaction {sup 56}Fe+p was investigated in inverse kinematics with regard to complete identification of the heavy residues. A ring imaging Cerenkov counter was used for velocity measurements in the experimental setup located at GSI in Darmstadt. A new fast readout electronic was developed and has been operated successfully in the experiment. Momentum reconstruction was carried out with the ALADiN spectrometer and a new software package written for this purpose. Cross sections and velocity distributions for more than 100 mass separated isotopes could be extracted from the dataset and compared with empirical models and other spallation experiments. The experiences gained in this experiment will be used for systematic improvements in the setup of the new spectrometer R3B at FAIR. (orig.)

  1. Transmutation of 126Sn in spallation targets of accelerator-driven systems

    International Nuclear Information System (INIS)

    Han, Chi Young; Saito, Masaki; Sagara, Hiroshi

    2009-01-01

    The practical feasibility of 126 Sn transmutation in spallation targets of accelerator-driven systems was evaluated from the viewpoints of accumulation of radioactive spallation products and neutron production as well as transmutation amount of 126 Sn. A cylindrical liquid 126 Sn target whose length depends on proton beam energy was described, based on a Pb-Bi target design of accelerator-driven system being developed in JAEA. A proton beam of 1.5 GeV-20 mA was estimated to give the transmutation rate of 126 Sn 6.4 kg/yr, which corresponds to the amount of 126 Sn annually discharged in 27 LWRs of 1 GWt and 33 GWd/THM. The equilibrium radioactivity of spallation products would reach 9% of that of 126 Sn transmuted in the spallation target, and the equilibrium toxicity would be just 3%. Some parametric analyses showed that the effective half-life of 126 Sn could be reduced through a proper reduction of the target size. The 126 Sn target was calculated to produce 40 neutrons per proton of 1.5 GeV and give a neutron spectrum very similar to that of the reference Pb-Bi target. As a result, the transmutation of 126 Sn in the spallation target has a high feasibility in terms of better transmutation performance and comparable target performance. (author)

  2. New scientific horizons with pulsed spallation neutron sources

    International Nuclear Information System (INIS)

    Carlile, C.J.; Finney, J.L.

    1991-01-01

    Pulsed spallation sources are not just another way of producing neutrons: the time structure of the neutron pulse has consequences which allow new scientific areas to be investigated and traditional areas to be explored afresh. In addition to the high epithermal neutron component traditionally associated with pulsed sources the recent development of cold neutron techniques at ISIS illustrates that very high energy and momentum resolutions can be achieved on pulsed sources over a surprisingly wide range. (orig.)

  3. Department of Energy review of the National Spallation Neutron Source Project

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1997-06-01

    A Department of Energy (DOE) review of the Conceptual Design Report (CDR) for the National Spallation Neutron Source (NSNS) was conducted. The NSNS will be a new high-power spallation neutron source; initially, it will operate at 1 megawatt (MW), but is designed to be upgradeable to significantly higher power, at lower cost, when accelerator and target technologies are developed for higher power. The 53-member Review Committee examined the projected cost, schedule, technical scope, and management structure described in the CDR. For each of the major components of the NSNS, the Committee determined that the project team had produced credible designs that can be expected to work well. What remains to be done is to integrate the design of these components. With the exception of the liquid mercury target, the NSNS Project will rely heavily on proven technologies and, thus, will face a relatively low risk to successful project completion. The Total Project Cost (TPC) presented to the Committee in the CDR was $1.266 billion in as-spent dollars. In general, the Committee felt that the laboratory consortium had presented a credible estimate for each of the major components but that value engineering might produce some savings. The construction schedule presented to the Committee covered six years beginning in FY 1999. The Committee questioned whether all parts of the project could be completed according to this schedule. In particular, the linac and the conventional facilities appeared to have overly optimistic schedules. The NSNS project team was encouraged to reexamine these activities and to consider a more conservative seven-year schedule. Another concern of the Committee was the management structure. In summary, the Committee felt that this Conceptual Design Report was a very credible proposal, and that there is a high probability for successful completion of this major project within the proposed budget, although the six-year proposed schedule may be optimistic.

  4. Department of Energy review of the National Spallation Neutron Source Project

    International Nuclear Information System (INIS)

    1997-06-01

    A Department of Energy (DOE) review of the Conceptual Design Report (CDR) for the National Spallation Neutron Source (NSNS) was conducted. The NSNS will be a new high-power spallation neutron source; initially, it will operate at 1 megawatt (MW), but is designed to be upgradeable to significantly higher power, at lower cost, when accelerator and target technologies are developed for higher power. The 53-member Review Committee examined the projected cost, schedule, technical scope, and management structure described in the CDR. For each of the major components of the NSNS, the Committee determined that the project team had produced credible designs that can be expected to work well. What remains to be done is to integrate the design of these components. With the exception of the liquid mercury target, the NSNS Project will rely heavily on proven technologies and, thus, will face a relatively low risk to successful project completion. The Total Project Cost (TPC) presented to the Committee in the CDR was $1.266 billion in as-spent dollars. In general, the Committee felt that the laboratory consortium had presented a credible estimate for each of the major components but that value engineering might produce some savings. The construction schedule presented to the Committee covered six years beginning in FY 1999. The Committee questioned whether all parts of the project could be completed according to this schedule. In particular, the linac and the conventional facilities appeared to have overly optimistic schedules. The NSNS project team was encouraged to reexamine these activities and to consider a more conservative seven-year schedule. Another concern of the Committee was the management structure. In summary, the Committee felt that this Conceptual Design Report was a very credible proposal, and that there is a high probability for successful completion of this major project within the proposed budget, although the six-year proposed schedule may be optimistic

  5. Molecular dynamics simulation of shock wave and spallation phenomena in metal foils irradiated by femtosecond laser pulse

    Science.gov (United States)

    Zhakhovsky, Vasily; Demaske, Brian; Inogamov, Nail; Oleynik, Ivan

    2010-03-01

    Femtosecond laser irradiation of metals is an effective technique to create a high-pressure frontal layer of 100-200 nm thickness. The associated ablation and spallation phenomena can be studied in the laser pump-probe experiments. We present results of a large-scale MD simulation of ablation and spallation dynamics developing in 1,2,3μm thick Al and Au foils irradiated by a femtosecond laser pulse. Atomic-scale mechanisms of laser energy deposition, transition from pressure wave to shock, reflection of the shock from the rear-side of the foil, and the nucleation of cracks in the reflected tensile wave, having a very high strain rate, were all studied. To achieve a realistic description of the complex phenomena induced by strong compression and rarefaction waves, we developed new embedded atom potentials for Al and Au based on cold pressure curves. MD simulations revealed the complex interplay between spallation and ablation processes: dynamics of spallation depends on the pressure profile formed in the ablated zone at the early stage of laser energy absorption. It is shown that the essential information such as material properties at high strain rate and spall strength can be extracted from the simulated rear-side surface velocity as a function of time.

  6. Observation of galactic cosmic ray spallation events from the SoHO mission 20-Year operation of LASCO

    Science.gov (United States)

    Koutchmy, S.; Tavabi, E.; Urtado, O.

    2018-05-01

    A shower of secondary Cosmic Ray (CR) particles is produced at high altitudes in the Earth's atmosphere, so the primordial Galactic Cosmic Rays (GCRs) are never directly measured outside the Earth magnetosphere and atmosphere. They approach the Earth and other planets in the complex pattern of rigidity's dependence, generally excluded by the magnetosphere. GCRs revealed by images of single nuclear reactions also called spallation events are described here. Such an event was seen on Nov. 29, 2015 using a unique LASCO C3 space coronagraph routine image taken during the Solar and Heliospheric Observatory (SoHO) mission observing uninterruptedly at the Lagrangian L1 point. The spallation signature of a GCR identified well outside the Earth's magnetosphere is obtained for the 1st time. The resulting image includes different diverging linear "tracks" of varying intensity, leading to a single pixel; this frame identifies the site on the silicon CCD chip of the coronagraph camera. There was no solar flare reported at that time, nor Coronal Mass Ejection (CME) and no evidence of optical debris around the spacecraft. More examples of smaller CR events have been discovered through the 20 years of continuous observations from SoHO. This is the first spallation event from a CR, recorded outside the Earth's magnetosphere. We evaluate the probable energy of these events suggesting a plausible galactic source.

  7. Astrophysical Li-7 as a product of big bang nucleosynthesis and galactic cosmic-ray spallation

    Science.gov (United States)

    Olive, Keith A.; Schramm, David N.

    1992-01-01

    The astrophysical Li-7 abundance is considered to be largely primordial, while the Be and B abundances are thought to be due to galactic cosmic ray (GCR) spallation reactions on top of a much smaller big bang component. But GCR spallation should also produce Li-7. As a consistency check on the combination of big bang nucleosynthesis and GCR spallation, the Be and B data from a sample of hot population II stars is used to subtract from the measured Li-7 abundance an estimate of the amount generated by GCR spallation for each star in the sample, and then to add to this baseline an estimate of the metallicity-dependent augmentation of Li-7 due to spallation. The singly reduced primordial Li-7 abundance is still consistent with big bang nucleosynthesis, and a single GCR spallation model can fit the Be, B, and corrected Li-7 abundances for all the stars in the sample.

  8. Fundamental physics possibilities at the European Spallation Source

    DEFF Research Database (Denmark)

    Klinkby, Esben Bryndt; Soldner, Torsten

    2016-01-01

    The construction of the European Spallation Source ESS is ongoing in Lund, Sweden. This new high power spallation source with its long-pulse structure opens up new possibilities for fundamental physics experiments. This paper focusses on two proposals for fundamental physics at the ESS: The ANNI...

  9. Isotopic production cross-sections and recoil velocities of spallation-fission fragments in the reaction 238U(1A GeV)+e

    CERN Document Server

    Pereira, J; Wlazlo, W; Benlliure, J; Casarejos, E; Armbruster, P; Bernas, M; Enqvist, T; Legrain, R; Leray, S; Rejmund, F; Mustapha, B; Schmidt, K.-H; Stéphan, C; Taïeb, J; Tassan-Got, L; Volant, C; Boudard, A; Czajkowski, S; 10.1103/PhysRevC.75.014602

    2007-01-01

    Fission fragments of 1A GeV 238U nuclei interacting with a deuterium target have been investigatedwith the Fragment Separator (FRS) at GSI (Darmstadt) by measuring their isotopicproduction cross-sections and recoil velocities. The results, along with those obtained recently forspallation-evaporation fragments, provide a comprehensive analysis of the spallation nuclear productionsin the reaction 238U(1A GeV)+d. Details about experiment performance, data reductionand results will be presented.

  10. Challenges and design solutions of the liquid hydrogen circuit at the European Spallation Source

    Energy Technology Data Exchange (ETDEWEB)

    Gallimore, S.; Nilsson, P.; Sabbagh, P.; Takibayev, A.; Weisend II, J. G. [European Spallation Source ESS AB, SE-22100 Lund (Sweden); Beßler, Y. [Forschungzentrum Jülich, Jülich (Germany); Klaus, M. [Technische Universität Dresden, Dresden (Germany)

    2014-01-29

    The European Spallation Source (ESS), Lund, Sweden will be a 5MW long-pulse neutron spallation research facility and will enable new opportunities for researchers in the fields of life sciences, energy, environmental technology, cultural heritage and fundamental physics. Neutrons are produced by accelerating a high-energy proton beam into a rotating helium-cooled tungsten target. These neutrons pass through moderators to reduce their energy to an appropriate range (< 5 meV for cold neutrons); two of which will use liquid hydrogen at 17 K as the moderating and cooling medium. There are several technical challenges to overcome in the design of a robust system that will operate under such conditions, not least the 20 kW of deposited heat. These challenges and the associated design solutions will be detailed in this paper.

  11. Toward high-efficiency and detailed Monte Carlo simulation study of the granular flow spallation target

    Science.gov (United States)

    Cai, Han-Jie; Zhang, Zhi-Lei; Fu, Fen; Li, Jian-Yang; Zhang, Xun-Chao; Zhang, Ya-Ling; Yan, Xue-Song; Lin, Ping; Xv, Jian-Ya; Yang, Lei

    2018-02-01

    The dense granular flow spallation target is a new target concept chosen for the Accelerator-Driven Subcritical (ADS) project in China. For the R&D of this kind of target concept, a dedicated Monte Carlo (MC) program named GMT was developed to perform the simulation study of the beam-target interaction. Owing to the complexities of the target geometry, the computational cost of the MC simulation of particle tracks is highly expensive. Thus, improvement of computational efficiency will be essential for the detailed MC simulation studies of the dense granular target. Here we present the special design of the GMT program and its high efficiency performance. In addition, the speedup potential of the GPU-accelerated spallation models is discussed.

  12. Research activities on structure materials of spallation neutron source at SINQ

    Energy Technology Data Exchange (ETDEWEB)

    Bauer, G.S.; Dai, Y. [Paul Scherrer Inst. (PSI), Villigen (Switzerland)

    1997-09-01

    With the growing interests on powerful spallation neutron sources, especially with liquid metal targets, and accelerator driven energy systems, spallation materials science and technology have been received wide attention. At SINQ, material research activities are focused on: a) liquid metal corrosion; b) radiation damage; and c) interaction of corrosion and radiation damage. (author) 1 fig., refs.

  13. Spallation radiation damage and the radiation damage facility at the LAMPF A-6 target station

    Energy Technology Data Exchange (ETDEWEB)

    Wechsler, M.S.; Sommer, W.F. (Los Alamos National Lab., NM (USA))

    1984-05-01

    A redesign of the Clinton P. Anderson Los Alamos Meson Physics Facility (LAMPF) A-6 Target Station is underway that will permit materials irradiations to be conducted in the proton beam and in the spallation neutron environment under more controlled conditions than has been possible heretofore. The protons of energy near 800 MeV and beam current approaching one mA are able to produce radiation damage rates (displacement production rates) as high as can be achieved in fission reactors, and the damage is uniform over macroscopic dimensions. The spallation neutrons have a degraded fission spectrum energy distribution, with the important admixture of a high energy tail up to 800 MeV. Irradiations in these radiation environments can be used to address important problems in the development of materials for fusion reactors. The redesign of the A-6 Target Station is described and plans for its use are discussed.

  14. Status of spallation neutron source

    Energy Technology Data Exchange (ETDEWEB)

    Oyama, Yukio [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

    1997-03-01

    Existing and planned facilities using proton accelerator driven spallation neutron source are reviewed. These include new project of neutron science proposed from Japan Atomic Energy Research Institute. The present status of facility requirement and accelerator technology leads us to new era of neutron science such as neutron scattering research and nuclear transmutation study using very intense neutron source. (author)

  15. Spallation neutron sources

    International Nuclear Information System (INIS)

    Fraser, J.S.; Bartholomew, G.A.

    1983-01-01

    The principles and theory of spallation neutron sources are outlined and a comparison is given with other types of neutron source. A summary of the available accelerator types for spallation neutron sources and their advantages and disadvantages is presented. Suitable target materials are discussed for specific applications, and typical target assemblies shown. (U.K.)

  16. Solid-state reactions to synthesize nanostructured lead selenide semiconductor powders by high-energy milling

    Energy Technology Data Exchange (ETDEWEB)

    Rojas-Chavez, H., E-mail: uu_gg_oo@yahoo.com.mx [Centro de Investigacion e Innovacion Tecnologica - IPN, Cerrada de CECATI s/n, Col. Santa Catarina, Del. Azcapotzalco (Mexico) and Centro de Investigacion en Ciencia Aplicada y Tecnologia Avanzada - IPN, Legaria 694, Col. Irrigacion, Del. Miguel Hidalgo (Mexico); Reyes-Carmona, F. [Facultad de Quimica - UNAM, Circuito de la Investigacion Cientifica s/n, C.U. Del. Coyoacan (Mexico); Jaramillo-Vigueras, D. [Centro de Investigacion e Innovacion Tecnologica - IPN, Cerrada de CECATI s/n, Col. Santa Catarina, Del. Azcapotzalco (Mexico)

    2011-10-15

    Highlights: {yields} PbSe synthesized from PbO instead of Pb powder do not require an inert atmosphere. {yields} During high-energy milling oxygen has to be chemically reduced from the lead oxide. {yields} Solid-state and solid-gas chemical reactions promote both solid and gaseous products. -- Abstract: Both solid-solid and gas-solid reactions have been traced during high-energy milling of Se and PbO powders under vial (P, T) conditions in order to synthesize the PbSe phase. Chemical and thermodynamic arguments are postulated to discern the high-energy milling mechanism to transform PbO-Se micropowders onto PbSe-nanocrystals. A set of reactions were evaluated at around room temperature. Therefore an experimental campaign was designed to test the nature of reactions in the PbO-Se system during high-energy milling.

  17. Solid-state reactions to synthesize nanostructured lead selenide semiconductor powders by high-energy milling

    International Nuclear Information System (INIS)

    Rojas-Chavez, H.; Reyes-Carmona, F.; Jaramillo-Vigueras, D.

    2011-01-01

    Highlights: → PbSe synthesized from PbO instead of Pb powder do not require an inert atmosphere. → During high-energy milling oxygen has to be chemically reduced from the lead oxide. → Solid-state and solid-gas chemical reactions promote both solid and gaseous products. -- Abstract: Both solid-solid and gas-solid reactions have been traced during high-energy milling of Se and PbO powders under vial (P, T) conditions in order to synthesize the PbSe phase. Chemical and thermodynamic arguments are postulated to discern the high-energy milling mechanism to transform PbO-Se micropowders onto PbSe-nanocrystals. A set of reactions were evaluated at around room temperature. Therefore an experimental campaign was designed to test the nature of reactions in the PbO-Se system during high-energy milling.

  18. Radioactive airborne species formed in the air in high energy accelerator tunnels

    International Nuclear Information System (INIS)

    Kondo, K.

    2005-01-01

    Many radioactive airborne species have been observed in the air of high energy accelerator tunnels during machine operation. Radiation protection against these induced airborne radioactivities is one of the key issues for radiation safety, especially at high-energy and high-intense proton accelerators such as the J-PARC (Japan Proton Accelerator Research Complex, Joint project of KEK and JAERI), which is now under construction at the TOKAI site of JAERI. Information on the chemical forms and particle sizes of airborne radioactivities is essential for the estimation of internal doses. For that purpose, the study on radioactive airborne species formed in the air of beam-line tunnels at high-energy accelerators have been extensively conducted by our group. For Be-7, Na-24, S-38, Cl-38,-39, C-11, and N-13, formed by various types of nuclear reactions including nuclear spallation reactions, their aerosol and gaseous fractions are determined by a filter technique. A parallel plate diffusion battery is used for the measurement of aerosol size distributions, and the formation of radioactive aerosols is explained by the attachment of radionuclides to ambient non-radioactive aerosols which are formed through radiation induced reactions. The chemical forms of gaseous species are also determined by using a selective collection method based on a filter technique. A review is given of the physico-chemical properties of these airborne radionuclides produced in the air of accelerator beam-line tunnels.

  19. Heavy ion reactions at high energies

    International Nuclear Information System (INIS)

    Jakobsson, Bo.

    1977-01-01

    A review on heavy ion experiments at energies >0.1GeV/nucleon is presented. Reaction cross-sections, isotope production cross-sections and pion production in nucleus-nucleus collisions are discussed. Some recent models for heavy ion reactions like the abrasion-ablation model, the fireball model and the different shock-wave models are also presented

  20. New neutron physics using spallation sources

    International Nuclear Information System (INIS)

    Bowman, C.D.

    1988-01-01

    The extraordinary neutron intensities available from the new spallation pulsed neutron sources open up exciting opportunities for basic and applied research in neutron nuclear physics. The energy range of neutron research which is being explored with these sources extends from thermal energies to almost 800 MeV. The emphasis here is on prospective experiments below 100 keV neutron energy using the intense neutron bursts produced by the Proton Storage Ring (PSR) at Los Alamos. 30 refs., 10 figs

  1. CFD Study of the Active Part of the HYPER LBE Spallation Target System

    International Nuclear Information System (INIS)

    Cho, Chung-ho; Tak, Nam-il; Lee, Yong-bum; Choi, Jae-Hyuk

    2007-01-01

    In an accelerator driven system (ADS), a high-energy proton beam impinges on a heavy metal target to produce spallation neutrons that are multiplied in a subcritical blanket. Therefore, the spallation target is one of the most important units of an ADS. A beam power of 15-25 MW is required for an operation of the HYPER system. But, the design of a 20 MW spallation target is very challenging because more than 60% of a beam power is deposited as heat in a small volume of a target system. LBE is preferred as the target material due to its high neutron production rate, effective heat removal, low melting point and vapor pressure, low neutron absorption and good radiation damage properties. In addition, it can be used simultaneously as a reactor coolant. Single hemi-spherical beam window is considered for the HYPER target. The beam window is a thin physical barrier to separate the vacuum space from the LBE. It is exposed to high thermal and irradiation loads, which affect its life time. The integrity of the beam window is crucial for a safe operation of the HYPER, for preventing the penetration of the radioactive spallation products into the accelerator island. Therefore, a sufficient cooling capability of the beam window is one of the key issues of the target design. In the previous study, a series of parametric thermal and mechanical studies were made for the optimization of the HYPER target. The optimized target has a 0.2 cm thick beam window with a diameter of 35 cm. Also, a 30 cm wide proton beam with a uniform beam distribution should be adopted for the spallation target of the HYPER. A dual injection tube is adopted to economize the LBE flow in the primary system. This paper presents the numerical studies on the optimized spallation target system. Several advanced turbulence models with different grid structures are investigated by using a commercial computational fluid dynamics (CFD) code CFX 5.7.1

  2. Calculation of displacement, gas, and transmutation production in stainless steel irradiated with spallation neutrons

    International Nuclear Information System (INIS)

    Wechsler, M.A.; Ramavarapu, R.; Daugherty, E.L.; Palmer, R.C.; Bullen, D.B.; Sommer, W.F.

    1993-01-01

    Calculations using the high-energy transport code LAHET have been made for the production of displacements, helium gas, and transmuted atoms for stainless steel (Fe-18 wt % Cr-10 wt % Ni) irradiated with spallation neutrons at energies of 100 to 1600 MeV. The damage energy cross section increased from about 250 to 350 b keV for increasing neutron energies from 100 to 1600 MeV with a spallation spectrum average of 281 barns-keV. For a displacement threshold energy of 33 eV, the corresponding spectrum-average displacement cross section is 3400 barns. The PKA spectrum was found to be fairly independent of the incident neutron energy, with an average damage energy of 0.25--0.30 MeV. The helium production cross section increased monotonically with increasing neutron energy, with a spectrum average of 0.32 barns. The maximum transmutation yield was observed near manganese (Z = 25), corresponding to a production cross section of about 0.2 barns. Relevance to fusion materials is discussed

  3. Sensitivity studies of the neutron multiplicity spectrum in the spallation of Pb targets

    International Nuclear Information System (INIS)

    Sinha, A.; Garg, S.B.; Srinivasan, M.

    1986-01-01

    The number of neutrons produced per incident proton in the spallation of Pb targets is of direct relevance to the design of accelerator breeders. The nuclear cascade initiated by high-energy protons in spallation targets is usually described by an intranuclear cascade evaporation (INCE) model. Even though this model describes various average nuclear properties of spallation targets fairly well, differential quantities such as energy spectra, angular spectra etc., are not reproduced within the limits of experimental uncertainty. One of the reasons for this is the uncertainty in the magnitude of the parameters involved in the model, notably the level density parameter Bsub(O) whose magnitude is quoted by different workers to be in the range of 8-20 MeV. The accuracy of Bsub(O) could be improved if we could experimentally determine a quantity which is much more sensitive to Bsub(O) than the average neutron yield. In this paper we discuss one such quantity, namely the neutron multiplicity spectrum (MS). We compute the MS due to the spallation of Pb targets of different sizes at proton energies of 1.5, 1.0 and 0.59 GeV using the Monte Carlo code HETC. It is noticed that for the 1.5 GeV proton case the probability P(ν) for leakage of ν neutrons for ν in the range of 60-65, changes by about 70% when Bsub(O) is varied from 8 to 20 MeV. The corresponding change in the average neutron yield is <20%. It is therefore suggested that an accurate measurement of the MS can serve as a useful tool to narrow down the range of uncertainty in the Bsub(O) parameter. (author)

  4. Measurement of nuclide cross-sections of spallation residues in 1 A GeV 238U + proton collisions

    International Nuclear Information System (INIS)

    Taieb, J.; Tassan-Got, L.; Bernas, M.; Mustapha, B.; Rejmund, F.; Stephan, C.; Schmidt, K.H.; Armbruster, P.; Benlliure, J.; Enqvist, T.; Boudard, A.; Legrain, R.; Leray, S.; Volant, C.; Wlazlo, W.; Casarejos, E.; Czajkowski, S.; Pravikoff, M.

    2003-02-01

    The production of heavy nuclides from the spallation-evaporation reaction of 238 U induced by 1 GeV protons was studied in inverse kinematics. The evaporation residues from tungsten to uranium were identified in-flight in mass and atomic number. Their production cross-sections and their momentum distributions were determined. The data are compared with empirical systematics. A comparison with previous results from the spallation of 208 Pb and 197 Au reveals the strong influence of fission in the spallation of 238 U. (orig.)

  5. Cross section measurement of residues produced in proton- and deuteron-induced spallation reactions on 93Zr at 105 MeV/u using the inverse kinematics method

    Directory of Open Access Journals (Sweden)

    Kawase Shoichiro

    2017-01-01

    Full Text Available Isotopic production cross sections in the proton- and deuteron-induced spallation reactions on 93Zr at an energy of 105 MeV/u were measured in inverse kinematics conditions for the development of realistic nuclear transmutation processes for long-lived fission products (LLFPs with neutron and light-ion beams. The experimental results were compared to the PHITS calculations describing the intra-nuclear cascade and evaporation processes. Although an overall agreement was obtained, a large overestimation of the production cross sections for the removal of a few nucleons was seen. A clear shell effect associated with the neutron magic number N = 50 was observed in the measured isotopic production yields of Zr and Y isotopes, which can be reproduced reasonably by the PHITS calculation.

  6. Spallation neutron source target station issues

    International Nuclear Information System (INIS)

    Gabriel, T.A.; Barnes, J.N.; Charlton, L.A.

    1996-01-01

    In many areas of physics, materials and nuclear engineering, it is extremely valuable to have a very intense source of neutrons so that the structure and function of materials can be studied. One facility proposed for this purpose is the National Spallation Neutron Source (NSNS). This facility will consist of two parts: (1) a high-energy (∼1 GeV) and high powered (∼ 1 MW) proton accelerator, and (2) a target station which converts the protons to low-energy (≤ 2 eV) neutrons and delivers them to the neutron scattering instruments. This paper deals with the second part, i.e., the design and development of the NSNS target station and the scientifically challenging issues. Many scientific and technical disciplines are required to produce a successful target station. These include engineering, remote handling, neutronics, materials, thermal hydraulics, and instrumentation. Some of these areas will be discussed

  7. Pressure and stress waves in a spallation neutron source mercury target generated by high-power proton pulses

    CERN Document Server

    Futakawa, M; Conrad, H; Stechemesser, H

    2000-01-01

    The international ASTE collaboration has performed a first series of measurements on a spallation neutron source target at the Alternating Gradient Synchrotron (AGS) in Brookhaven. The dynamic response of a liquid mercury target hit by high-power proton pulses of about 40 ns duration has been measured by a laser Doppler technique and compared with finite elements calculations using the ABAQUS code. It is shown that the calculation can describe the experimental results for at least the time interval up to 100 mu s after the pulse injection. Furthermore, it has been observed that piezoelectric pressure transducers cannot be applied in the high gamma-radiation field of a spallation target.

  8. Isotopic yields and kinetic energies of primary residues in 1 A GeV 208Pb + p reactions

    International Nuclear Information System (INIS)

    Enqvist, T.; Wlazlo, W.; Armbruster, P.

    2000-09-01

    The production of primary residual nuclei in the reaction 1 A GeV 208 Pb on proton has been studied by measuring isotopic distributions for all elements from titanium (Z=22) to lead (Z=82). Kinematical properties of the residues were also determined and used to disentangle the relevant reaction mechanisms, spallation (projectile fragmentation) and fission. The fragment separator FRS at GSI, Darmstadt, was used to separate and identify the reaction products. The measured production cross sections are highly relevant for the design of accelerator-driven subcritical reactors and for the planning of future radioactive-beam facilities. (orig.)

  9. Modelling of an experiment for the study of neutron spallation source at JINR

    International Nuclear Information System (INIS)

    Kumawat, Harphool; Goyal, Uttam; Kumar, V.; Barashenkov, V.S.

    2002-01-01

    Intense neutron spallation source (INSS) is a necessary requirement of accelerator driven sub-critical systems. INSS are proposed to be generated using the high current proton beams. Some studies are conducted for the neutron flux, transmutation rates and energy gains and a larger number of related experiments are being planned

  10. Isobaric yield curves at A=72 from the spallation of medium mass isotopes by intermediate energy protons

    International Nuclear Information System (INIS)

    Tobin, M.J.; Karol, P.J.; Department of Chemistry, Carnegie-Mellon University, Pittsburgh, Pennsylvania 15213)

    1989-01-01

    Cross sections of radionuclides in the A∼72 mass region produced by the interaction 800 MeV protons with 89 Y, /sup 92,96,100/Mo, and 130 Te were measured. Particular emphasis was paid to the measurement of short-lived products far from β stability. The cross sections were used to generate isobaric yield curves at A=72. Precise characterization of these curves showed that the distribution parameters (mean, standard deviation, skewness) vary in a regular fashion with target N/Z. For 89 Y, relative isobaric curves produced by 500 and 800 MeV protons were found to be identical within experimental error. The yield distributions for the /sup 92,96,100/Mo targets also scaled with those from an earlier alpha-induced spallation study. These findings lend strong support to the argument that the spallation mechanism is independent of projectile energy and target composition

  11. Measured radionuclide production from copper, gold and lead spallation targets

    Energy Technology Data Exchange (ETDEWEB)

    Parish, T.A.; Belian, A.P. [Texas A & M Univ., College Station, TX (United States)

    1995-10-01

    Spallation target materials are chosen so as to produce large numbers of neutrons while at the same time avoiding the creation of long-lived radioactive wastes. While there has been considerable research to determine the number of neutrons produced per incident particle for various target materials, there has been less effort to precisely quantify the types and amounts of radionuclides produced. Accurate knowledge of the radioactive species produced by spallation reactions is important for specifying waste disposal criteria for targets. In order to verify the production rates calculated by LAHET, a study has been conducted using the Texas A&M University (TAMU) Cyclotron to measure radionuclide yields from copper, gold, and lead targets.

  12. Rationale for a spallation neutron source target system test facility at the 1-MW Long-Pulse Spallation Source

    International Nuclear Information System (INIS)

    Sommer, W.F.

    1995-12-01

    The conceptual design study for a 1-MW Long-Pulse Spallation Source at the Los Alamos Neutron Science Center has shown the feasibility of including a spallation neutron test facility at a relatively low cost. This document presents a rationale for developing such a test bed. Currently, neutron scattering facilities operate at a maximum power of 0.2 MW. Proposed new designs call for power levels as high as 10 MW, and future transmutation activities may require as much as 200 MW. A test bed will allow assessment of target neutronics; thermal hydraulics; remote handling; mechanical structure; corrosion in aqueous, non-aqueous, liquid metal, and molten salt systems; thermal shock on systems and system components; and materials for target systems. Reliable data in these areas are crucial to the safe and reliable operation of new high-power facilities. These tests will provide data useful not only to spallation neutron sources proposed or under development, but also to other projects in accelerator-driven transmutation technologies such as the production of tritium

  13. GEANT4 simulations of the n{sub T}OF spallation source and their benchmarking

    Energy Technology Data Exchange (ETDEWEB)

    Lo Meo, S. [Research Centre ' ' Ezio Clementel' ' , ENEA, Bologna (Italy); Section of Bologna, INFN, Bologna (Italy); Cortes-Giraldo, M.A.; Lerendegui-Marco, J.; Guerrero, C.; Quesada, J.M. [Universidad de Sevilla, Facultad de Fisica, Sevilla (Spain); Massimi, C.; Vannini, G. [Section of Bologna, INFN, Bologna (Italy); University of Bologna, Physics and Astronomy Dept. ' ' Alma Mater Studiorum' ' , Bologna (Italy); Barbagallo, M.; Colonna, N. [INFN, Section of Bari, Bari (Italy); Mancusi, D. [CEA-Saclay, DEN, DM2S, SERMA, LTSD, Gif-sur-Yvette CEDEX (France); Mingrone, F. [Section of Bologna, INFN, Bologna (Italy); Sabate-Gilarte, M. [Universidad de Sevilla, Facultad de Fisica, Sevilla (Spain); European Organization for Nuclear Research (CERN), Geneva (Switzerland); Vlachoudis, V. [European Organization for Nuclear Research (CERN), Geneva (Switzerland); Collaboration: The n_TOF Collaboration

    2015-12-15

    Neutron production and transport in the spallation target of the n{sub T}OF facility at CERN has been simulated with GEANT4. The results obtained with different models of high-energy nucleon-nucleus interaction have been compared with the measured characteristics of the neutron beam, in particular the flux and its dependence on neutron energy, measured in the first experimental area. The best agreement at present, within 20% for the absolute value of the flux, and within few percent for the energy dependence in the whole energy range from thermal to 1 GeV, is obtained with the INCL++ model coupled with the GEANT4 native de-excitation model. All other available models overestimate by a larger factor, of up to 70%, the n{sub T}OF neutron flux. The simulations are also able to accurately reproduce the neutron beam energy resolution function, which is essentially determined by the moderation time inside the target/moderator assembly. The results here reported provide confidence on the use of GEANT4 for simulations of spallation neutron sources. (orig.)

  14. Use of a GDMS for high-energy reaction data

    International Nuclear Information System (INIS)

    Moorhead, W.G.

    1978-01-01

    At CERN, data on high-energy reactions is being compiled using a Generalized Data Management System. The GDMS is a stand-alone system designed for administrative and engineering applications. The Data Base at present contains about 20,000 cross-section values, each linked to a description of the corresponding reaction, and the publication from which the value was derived. The immediate objective is to produce the widely circulated Compilation Reports, and the standard Report Generator of the GDMS is being used for this. Direct retrieval is also possible

  15. Production of complex particles in low energy spallation and in fragmentation reactions by in-medium random clusterization

    International Nuclear Information System (INIS)

    Lacroix, D.; Durand, D.

    2005-09-01

    Rules for in-medium complex particle production in nuclear reactions are proposed. These rules have been implemented in two models to simulate nucleon-nucleus and nucleus-nucleus reactions around the Fermi energy. Our work emphasizes the effect of randomness in cluster formation, the importance of the nucleonic Fermi motion as well as the role of conservation laws. The concepts of total available phase-space and explored phase-space under constraint imposed by the reaction are clarified. The compatibility of experimental observations with a random clusterization is illustrated in a schematic scenario of a proton-nucleus collision. The role of randomness under constraint is also illustrated in the nucleus-nucleus case. (authors)

  16. Standard Test Method for Measuring Fast-Neutron Reaction Rates by Radioactivation of Niobium

    CERN Document Server

    American Society for Testing and Materials. Philadelphia

    2008-01-01

    1.1 This test method describes procedures for measuring reaction rates by the activation reaction 93Nb(n,n′)93mNb. 1.2 This activation reaction is useful for monitoring neutrons with energies above approximately 0.5 MeV and for irradiation times up to about 30 years. 1.3 With suitable techniques, fast-neutron reaction rates for neutrons with energy distribution similar to fission neutrons can be determined in fast-neutron fluences above about 1016cm−2. In the presence of high thermal-neutron fluence rates (>1012cm−2·s−1), the transmutation of 93mNb due to neutron capture should be investigated. In the presence of high-energy neutron spectra such as are associated with fusion and spallation sources, the transmutation of 93mNb by reactions such as (n,2n) may occur and should be investigated. 1.4 Procedures for other fast-neutron monitors are referenced in Practice E 261. 1.5 Fast-neutron fluence rates can be determined from the reaction rates provided that the appropriate cross section information ...

  17. Spallator and APEX nuclear fuel cycle: a new option for nuclear power

    International Nuclear Information System (INIS)

    Steinberg, M.

    1982-01-01

    A new nuclear fuel cycle is described which provides a long term supply of nuclear fuel for the thermal LWR nuclear power reactors and eliminates the need for long-term storage of radioactive waste. Fissile fuel is produced by the Spallator which depends on the production of spallation neutrons by the interaction of high-energy (1 to 2 GeV) protons on a heavy-metal target. The neutrons are absorbed in a surrounding natural-uranium or thorium blanket in which fissile Pu-239 to U-233 is produced. Advances in linear accelerator technology makes it possible to design and construct a high-beam-current continuous-wave proton linac for production purposes. The target is similar to a sub-critical reactor and produces heat which is converted to electricity for supplying the linac. The Spallator is a self-sufficient fuel producer, which can compete with the fast breeder. The APEX fuel cycle depends on recycling the transuranics and long-lived fission products while extracting the stable and short-lived fission products when reprocessing the fuel. Transmutation and decay within the fuel cycle and decay of short-lived fission products external to the fuel cycle eliminates the need for long-term geological age shortage of fission-product waste

  18. Spallator and APEX nuclear fuel cycle: a new option for nuclear power

    Energy Technology Data Exchange (ETDEWEB)

    Steinberg, M.

    1982-01-01

    A new nuclear fuel cycle is described which provides a long term supply of nuclear fuel for the thermal LWR nuclear power reactors and eliminates the need for long-term storage of radioactive waste. Fissile fuel is produced by the Spallator which depends on the production of spallation neutrons by the interaction of high-energy (1 to 2 GeV) protons on a heavy-metal target. The neutrons are absorbed in a surrounding natural-uranium or thorium blanket in which fissile Pu-239 to U-233 is produced. Advances in linear accelerator technology makes it possible to design and construct a high-beam-current continuous-wave proton linac for production purposes. The target is similar to a sub-critical reactor and produces heat which is converted to electricity for supplying the linac. The Spallator is a self-sufficient fuel producer, which can compete with the fast breeder. The APEX fuel cycle depends on recycling the transuranics and long-lived fission products while extracting the stable and short-lived fission products when reprocessing the fuel. Transmutation and decay within the fuel cycle and decay of short-lived fission products external to the fuel cycle eliminates the need for long-term geological age shortage of fission-product waste.

  19. Measurements of neutron spallation cross section. 2

    Energy Technology Data Exchange (ETDEWEB)

    Kim, E.; Nakamura, T. [Tohoku Univ., Sendai (Japan). Cyclotron and Radioisotope Center; Imamura, M.; Nakao, N.; Shibata, S.; Uwamino, Y.; Nakanishi, N.; Tanaka, Su.

    1997-03-01

    Neutron spallation cross section of {sup 59}Co(n,xn){sup 60-x}Co, {sup nat}Cu(n,sp){sup 56}Mn, {sup nat}Cu(n,sp){sup 58}Co, {sup nat}Cu(n,xn){sup 60}Cu, {sup nat}Cu(n,xn){sup 61}Cu and {sup nat}Cu(n,sp){sup 65}Ni was measured in the quasi-monoenergetic p-Li neutron fields in the energy range above 40 MeV which have been established at three AVF cyclotron facilities of (1) INS of Univ. of Tokyo, (2) TIARA of JAERI and (3) RIKEN. Our experimental data were compared with the ENDF/B-VI high energy file data by Fukahori and the calculated cross section data by Odano. (author)

  20. Neutron Production by Muon Spallation I: Theory

    International Nuclear Information System (INIS)

    Luu, T; Hagmann, C

    2006-01-01

    We describe the physics and codes developed in the Muon Physics Package. This package is a self-contained Fortran90 module that is intended to be used with the Monte Carlo package MCNPX. We calculate simulated energy spectra, multiplicities, and angular distributions of direct neutrons and pions from muon spallation

  1. Using (n,xnγ) reactions to probe collective nuclear structure

    International Nuclear Information System (INIS)

    Yates, S.W.; Brown, T.B.; Warr, N.; Hannant, C.D.

    2000-01-01

    Complete text of publication follows. The (n,n'γ) reaction has been utilized at the University of Kentucky accelerator laboratory for many years to study the structure of stable nuclei (1,2). Through the use of γ-ray excitation function and angular distribution measurements, detailed level schemes of stable nuclei can be established. In recent years, the Doppler-shift attenuation method (DSAM) has been applied following the inelastic neutron scattering reaction to determine the lifetimes of nuclear states (3), and collimated neutron 'beams' have been employed in γ-γ coincidence measurements with an array of HPGe detectors in a close geometry (4,5). Recently, γ-ray detection facilities (6,7) for reactions induced by spallation neutrons, with energies of several hundred MeV, have become available at the Los Alamos Neutron Science Center (LANSCE), and initial measurements indicate that a large variety of reactions are possible. Evidence has been obtained for reactions with as many as 27 particles emitted (7). While the mechanisms of such reactions may be of interest, the primary spectroscopic advantage of utilizing higher-energy neutrons appears to be that neutron-rich nuclei which are not normally available for study with fusion-evaporation reactions can be accessed. As a complement to these measurements with very energetic neutrons, (n2nγ) and (n,3nγ) reaction studies have been explored with neutrons from the 2 H(d,n) and 3 H(d,n) reactions and the facilities at the University of Kentucky. Neutron energies as high as 22 MeV have been employed. Initial evaluations have focussed on data from the 186 W(n,2nγ) 185 W and 186 W(n,3nγ) 184 W reactions and indicate that a great deal of information can be obtained. The advantages of these measurements, as well as comparisons with data from reactions with spallation neutrons, will be presented. This work was supported under grant PHY-9803784 from the U.S. National Science Foundation. (author)

  2. Synthesis of neutron-rich transuranic nuclei in fissile spallation targets

    Energy Technology Data Exchange (ETDEWEB)

    Mishustin, Igor, E-mail: mishustin@fias.uni-frankfurt.de [Frankfurt Institute for Advanced Studies, J.-W. Goethe University, 60438 Frankfurt am Main (Germany); “Kurchatov Institute”, National Research Center, 123182 Moscow (Russian Federation); Malyshkin, Yury, E-mail: malyshkin@fias.uni-frankfurt.de [Frankfurt Institute for Advanced Studies, J.-W. Goethe University, 60438 Frankfurt am Main (Germany); Institute for Nuclear Research, Russian Academy of Sciences, 117312 Moscow (Russian Federation); Pshenichnov, Igor, E-mail: pshenich@fias.uni-frankfurt.de [Frankfurt Institute for Advanced Studies, J.-W. Goethe University, 60438 Frankfurt am Main (Germany); Institute for Nuclear Research, Russian Academy of Sciences, 117312 Moscow (Russian Federation); Greiner, Walter [Frankfurt Institute for Advanced Studies, J.-W. Goethe University, 60438 Frankfurt am Main (Germany)

    2015-04-15

    A possibility of synthesizing neutron-rich superheavy elements in spallation targets of Accelerator Driven Systems (ADS) is considered. A dedicated software called Nuclide Composition Dynamics (NuCoD) was developed to model the evolution of isotope composition in the targets during a long-time irradiation by intense proton and deuteron beams. Simulation results show that transuranic elements up to {sup 249}Bk can be produced in multiple neutron capture reactions in macroscopic quantities. However, the neutron flux achievable in a spallation target is still insufficient to overcome the so-called fermium gap. Further optimization of the target design, in particular, by including moderating material and covering it by a reflector could turn ADS into an alternative source of transuranic elements in addition to nuclear fission reactors.

  3. The RADEX facility as a tool for studies of radiation damage under proton and spallation neutron irradiation

    Energy Technology Data Exchange (ETDEWEB)

    Koptelov, E.A.; Lebedev, S.G.; Matveev, V.A.; Sobolevsky, N.M. [Institute for Nuclear Research of Russian Academy of Sciences, Moscow (Russian Federation); Strebkov, Yu.S.; Subbotin, A.V. [Research and Development Institute of Power Engineering, Moscow (Russian Federation)

    2001-03-01

    We present results of numerical modeling for processes of primary protons and spallation neutrons interactions with structural materials at the RADiation EXperiment facility of the Neutron Complex. The installation has a vertical irradiation channel inside the beam stop for horizontally incident protons with energies up to 600 MeV of the Moscow Meson Factory of the INR (Institute for Nuclear Research) RAS (Russian Academy of Science). The calculations are based on a set of computer codes SHIELD and RADDAM, which were developed in the INR RAS and give data on point defect generation by irradiation, rate of accumulation of H and He atoms produced in nuclear reactions, energetic spectra of primary knocked-off atoms in collision displacements, temperature of samples under irradiation. Different positions of the channel, which are available by rotation of a target relatively the vertical axis for angles 0, 60, 120 and 180 degrees to the proton beam direction, are considered. Changes of irradiation damage parameters due to various inputs of primary protons and spallation neutrons at different target orientations are demonstrated. It is shown also that the spallation neutron facility RADEX may provide with perspective experimental possibilities for modeling of irradiation conditions for fusion reactors ITER and DEMO. (author)

  4. Influence of the nuclear level density on the odd-even staggering in 56Fe+p spallation at energies from 300 to 1500 MeV/nucleon

    Science.gov (United States)

    Su, Jun; Zhu, Long; Guo, Chenchen

    2018-05-01

    Background: Special attention has been paid to study the shell effect and odd-even staggering (OES) in the nuclear spallation. Purpose: In this paper, we investigate the influence of the nuclear level density on the OES in the 56Fe+p spallations at energies from 300 to 1500 MeV/nucleon. Method: The isospin-dependent quantum molecular dynamics (IQMD) model is applied to produce the highly excited and equilibrium remnants, which is then de-excited using the statistical model gemini. The excitation energy of the heaviest hot fragments is applied to match the IQMD model with the gemini model. In the gemini model, the statistical description of the evaporation are based on the Hauser-Feshbach formalism, in which level density prescriptions are applied. Results: By investigating the OES of the excited pre-fragments, it is found that the OES originates at the end of the decay process when the excitation energy is close to the nucleon-emission threshold energy, i.e., the smaller value of the neutron separation energy and proton separation energy. The strong influence of level density on the OES is noticed. Two types of the nuclear level densities, the discrepancy of which is only about 7% near the nucleon emission threshold energy, are used in the model. However, the calculated values of the OES differ by the factor of 3 for the relevant nuclei. Conclusions: It is suggested that, although the particle-separation energies play a key role in determining the OES, the level density at excitation energy lower than the particle-separation energies should be taken into consideration

  5. An investigation of fission models for high-energy radiation transport calculations

    International Nuclear Information System (INIS)

    Armstrong, T.W.; Cloth, P.; Filges, D.; Neef, R.D.

    1983-07-01

    An investigation of high-energy fission models for use in the HETC code has been made. The validation work has been directed checking the accuracy of the high-energy radiation transport computer code HETC to investigate the appropriate model for routine calculations, particularly for spallation neutron source applications. Model calculations are given in terms of neutron production, fission fragment energy release, and residual nuclei production for high-energy protons incident on thin uranium targets. The effect of the fission models on neutron production from thick uranium targets is also shown. (orig.)

  6. A linac for the Spallation Neutron Source

    International Nuclear Information System (INIS)

    Jason, A.J.

    1998-01-01

    The Spallation Neutron Source Project (SNS), to be constructed at Oak Ridge National Laboratory, accelerates H - ions to an energy of 1.0 GeV with an average current of 1-mA for injection into an accumulator ring that produces the short intense burst of protons needed for the spallation-neutron source. The linac will be the most intense source of H - ions and as such requires advanced design techniques to meet project technical goals. In particular, low beam loss is stressed for the chopped beam placing strong requirements on the beam dynamics and linac construction. Additionally, the linac is to be upgraded to the 2- and 4-MW beam-power levels with no increase in duty factor. The author gives an overview of the linac design parameters and design choices made

  7. Moisture-Induced TBC Spallation on Turbine Blade Samples

    Science.gov (United States)

    Smialek, James

    2011-01-01

    Delayed failure of TBCs is a widely observed laboratory phenomenon, although many of the early observations went unreported. The weekend effect or DeskTop Spallation (DTS) is characterized by initial survival of a TBC after accelerated laboratory thermal cycling, then failure by exposure to ambient humidity or water. Once initiated, failure can occur quite dramatically in less than a second. To this end, the water drop test and digital video recordings have become useful techniques in studies at NASA (Smialek, Zhu, Cuy), DECHMA (Rudolphi, Renusch, Schuetze), and CNRS Toulouse/SNECMA (Deneux, Cadoret, Hervier, Monceau). In the present study the results for a commercial turbine blade, with a standard EB-PVD 7YSZ TBC top coat and Pt-aluminide diffusion bond coat are reported. Cut sections were intermittently oxidized at 1100, 1150, and 1200 C and monitored by weight change and visual appearance. Failures were distributed widely over a 5-100 hr time range, depending on temperature. At some opportune times, failure was captured by video recording, documenting the appearance and speed of the moisture-induced spallation process. Failure interfaces exhibited alumina scale grains, decorated with Ta-rich oxide particles, and alumina inclusions as islands and streamers. The phenomenon is thus rooted in moisture-induced delayed spallation (MIDS) of the alumina scale formed on the bond coat. In that regard, many studies show the susceptibility of alumina scales to moisture, as long as high strain energy and a partially exposed interface exist. The latter conditions result from severe cyclic oxidation conditions, which produce a highly stressed and partially damaged scale. In one model, it has been proposed that moisture reacts with aluminum in the bond coat to release hydrogen atoms that embrittle the interface. A negative synergistic effect with interfacial sulfur is also invoked.

  8. Technology and science at a high-power spallation source: Proceedings

    Energy Technology Data Exchange (ETDEWEB)

    1994-01-01

    These proceedings cover many aspects of the usefulness of spallation neutrons. Nine different areas are considered: surfaces and interfaces, engineering, materials science, polymers and complex fluids, chemistry, structural biology, nuclear engineering and radiation effects, condensed matter physics and fundamental physics.

  9. Technology and science at a high-power spallation source: Proceedings

    International Nuclear Information System (INIS)

    1994-01-01

    These proceedings cover many aspects of the usefulness of spallation neutrons. Nine different areas are considered: surfaces and interfaces, engineering, materials science, polymers and complex fluids, chemistry, structural biology, nuclear engineering and radiation effects, condensed matter physics and fundamental physics

  10. Design of an experimental device dedicated to the measurement of spallation reactions; Mise au point d'un dispositif experimental pour des mesures exclusives des reactions de spallation

    Energy Technology Data Exchange (ETDEWEB)

    Lafriakh, A

    2005-12-15

    Spallation mechanisms are not yet completely understood, especially because of the difficulty of experimentally disentangling the effects of the different steps of the reaction. In order to understand these mechanisms, we have developed a new experimental device able to perform inclusive measurements. We propose a detection system based on a combination of ionization chambers and proportional counters and on a wall of plastic scintillators to measure light charged particles. In particular the detection of light charged particles is described in detail. In order to validate our device, we have compared our preliminary results obtained on the Fe{sup 56} + p system at 1 GeV/u with inclusive measurements previously obtained at the FRS spectrometer of the GSI facility. A comparison of charge differential cross section shows reasonable agreement. However, our new device allowed extension of those measurements down to Z = 1 and Z = 2. These cross sections are important for material damage studies. Taking into account our error brackets, the evolution of mean longitudinal velocities with respect to residue masses is comparable to that obtained at the FRS. These first results, although preliminary, allow us to validate our experimental device. It is now possible to exploit the strong points of our exclusive measurements, namely correlations between different measured observables. Finally, experimental problems encountered will be taken into account in the future experimental programs, in order to ensure the best measurements conditions.

  11. Nuclear spallation of cosmic ray nuclei in the interstellar medium

    International Nuclear Information System (INIS)

    Raisbeck, G.

    1974-01-01

    Nuclear spallation of cosmic rays during propagation is qualitatively reviewed. After the problem is defined, a discussion is presented of the relevant information obtainable from studying nuclear reactions, specifically, quantity and distribution of traversed matter, time and place of propagation, and source composition. Comments are offered on the cross sections and nuclear reactions that are critical for a complete understanding in this area. This is followed by a brief look at the present status of research and possibilities for further work using the Bevalac. (U.S.)

  12. Intermediate and high energy nuclear reactions at the hadronic structural level

    Energy Technology Data Exchange (ETDEWEB)

    Slowinski, B [Institute of Physics, Warsaw, University of Technology, Poland, Institute of Atomic Energy, Swierk, (Poland)

    1997-12-31

    Form tens of MeV to several hundred of GeV is stretched out quite a large interval of energy when the interaction between hadrons (for instance, pion/nucleon-nucleus and nucleus-nucleus reactions) can be described by the considerably simplified way with still acceptable accuracy. This happens because in this energy region hadrons (i.e. pions, nucleons etc.) remain quasiparticles of nuclear matter mostly without revealing any internal structure, their de Broglie`s wavelength is much shorter as compared to the average intranuclear nucleon`s distance, and the energy transfers in the reaction are, on the average, significantly greater than the binding energy of nucleons inside nuclei. Consequently an approach to the analysis of these phenomena based on simple geometric and probabilistic considerations is justifiable, especially for many practical purposes, in particular, for shielding and dosimetric estimations, material behaviour prediction, as well as for the approximate evaluation of electronuclear breeding effects in different composites of target materials, for nuclear passivation problems and so on. In this work basic physical reasons of such a simplified picture of intermediate and high energy nuclear reactions are presented. The most usual phenomenological models of hadronic multiple emission/production and recent results of the cascade evaporation type models, are also discussed. 2 figs.

  13. High energy reactions in normal metabolism and ageing of animals

    International Nuclear Information System (INIS)

    Avdonina, E.N.; Nesmeyanov, N.

    1983-01-01

    Processes involving reactions on highly excited states are thought to be of great importance for normal metabolism and aging. Excess energy of the organism is transferred to result in the formation of highly excited states of macromolecules. UV, visible light or ionizing radiation created partially by the organism itself can change metabolic process rates. According to the authors, aging is associated with the defects of macromolecules owing to high energy processes. Gerontological changes in biological materials result from the elimination of low molecular weight molecules and from the formation of unsaturated compounds. Crosslinking of the compounds, accumulation of collagen and connective tissues, the energetic overload of the organism are listed as important features of aging. (V.N.)

  14. The thermal triple-axis-spectrometer EIGER at the continuous spallation source SINQ

    Energy Technology Data Exchange (ETDEWEB)

    Stuhr, U., E-mail: uwe.stuhr@psi.ch [Laboratory of Neutron Scattering and Imaging, Paul Scherrer Institute, 5232 Villigen PSI (Switzerland); Roessli, B.; Gvasaliya, S. [Laboratory of Neutron Scattering and Imaging, Paul Scherrer Institute, 5232 Villigen PSI (Switzerland); Rønnow, H.M. [Laboratory for Quantum Magnetism, Institute of Physics, Ecole Polytechnique Féderale de Lausanne (EPFL), CH-1015 Lausanne (Switzerland); Filges, U.; Graf, D.; Bollhalder, A.; Hohl, D.; Bürge, R.; Schild, M.; Holitzner, L.; Kaegi, C.; Keller, P.; Mühlebach, T. [Laboratory for Scientific Development and Novel Materials, Paul Scherrer Institute, 5232 Villigen PSI (Switzerland)

    2017-05-01

    EIGER is the new thermal triple-axis-spectrometer at the continuous spallation SINQ at PSI. The shielding of the monochromator consists only of non- or low magnetizable materials, which allows the use of strong magnetic fields with the instrument. This shielding reduces the high energy neutron contamination to a comparable level of thermal spectrometers at reactor sources. The instrument design, the performance and first results of the spectrometer are presented.

  15. HYSPEC : A CRYSTAL TIME OF FLIGHT HYBRID SPECTROMETER FOR THE SPALLATION NEUTRON SOURCE

    International Nuclear Information System (INIS)

    SHAPIRO, S.M.; ZALIZNYAK, I.A.

    2002-01-01

    This document lays out a proposal by the Instrument Development Team (IDT) composed of scientists from leading Universities and National Laboratories to design and build a conceptually new high-flux inelastic neutron spectrometer at the pulsed Spallation Neutron Source (SNS) at Oak Ridge. This instrument is intended to supply users of the SNS and scientific community, of which the IDT is an integral part, with a platform for ground-breaking investigations of the low-energy atomic-scale dynamical properties of crystalline solids. It is also planned that the proposed instrument will be equipped with a polarization analysis capability, therefore becoming the first polarized beam inelastic spectrometer in the SNS instrument suite, and the first successful polarized beam inelastic instrument at a pulsed spallation source worldwide. The proposed instrument is designed primarily for inelastic and elastic neutron spectroscopy of single crystals. In fact, the most informative neutron scattering studies of the dynamical properties of solids nearly always require single crystal samples, and they are almost invariably flux-limited. In addition, in measurements with polarization analysis the available flux is reduced through selection of the particular neutron polarization, which puts even more stringent limits on the feasibility of a particular experiment. To date, these investigations have mostly been carried out on crystal spectrometers at high-flux reactors, which usually employ focusing Bragg optics to concentrate the neutron beam on a typically small sample. Construction at Oak Ridge of the high-luminosity spallation neutron source, which will provide intense pulsed neutron beams with time-averaged fluxes equal to those at medium-flux reactors, opens entirely new opportunities for single crystal neutron spectroscopy. Drawing upon experience acquired during decades of studies with both crystal and time-of-flight (TOF) spectrometers, the IDT has developed a conceptual

  16. HYSPEC : A CRYSTAL TIME OF FLIGHT HYBRID SPECTROMETER FOR THE SPALLATION NEUTRON SOURCE.

    Energy Technology Data Exchange (ETDEWEB)

    SHAPIRO,S.M.; ZALIZNYAK,I.A.

    2002-12-30

    This document lays out a proposal by the Instrument Development Team (IDT) composed of scientists from leading Universities and National Laboratories to design and build a conceptually new high-flux inelastic neutron spectrometer at the pulsed Spallation Neutron Source (SNS) at Oak Ridge. This instrument is intended to supply users of the SNS and scientific community, of which the IDT is an integral part, with a platform for ground-breaking investigations of the low-energy atomic-scale dynamical properties of crystalline solids. It is also planned that the proposed instrument will be equipped with a polarization analysis capability, therefore becoming the first polarized beam inelastic spectrometer in the SNS instrument suite, and the first successful polarized beam inelastic instrument at a pulsed spallation source worldwide. The proposed instrument is designed primarily for inelastic and elastic neutron spectroscopy of single crystals. In fact, the most informative neutron scattering studies of the dynamical properties of solids nearly always require single crystal samples, and they are almost invariably flux-limited. In addition, in measurements with polarization analysis the available flux is reduced through selection of the particular neutron polarization, which puts even more stringent limits on the feasibility of a particular experiment. To date, these investigations have mostly been carried out on crystal spectrometers at high-flux reactors, which usually employ focusing Bragg optics to concentrate the neutron beam on a typically small sample. Construction at Oak Ridge of the high-luminosity spallation neutron source, which will provide intense pulsed neutron beams with time-averaged fluxes equal to those at medium-flux reactors, opens entirely new opportunities for single crystal neutron spectroscopy. Drawing upon experience acquired during decades of studies with both crystal and time-of-flight (TOF) spectrometers, the IDT has developed a conceptual

  17. A comparison between short pulse spallation source and long pulse spallation source

    Energy Technology Data Exchange (ETDEWEB)

    Aizawa, Kazuya; Watanabe, Noboru; Suzuki, Jun-ichi; Niimura, Nobuo; Morii, Yukio; Katano, Susumu; Osakabe, Toyotaka; Teshigawara, Makoto [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment; Mezei, F.

    1997-11-01

    The performance for a 5 MW short pulse spallation source (SPSS) and a 4.5 MW long pulse spallation source (LPSS) in a JAERI program which is based on the availability of a 1.5 GeV superconducting linac with a 30 mA peak current for both proton and H{sup -} beams is discussed. We have examined the superiority of SPSS to LPSS. While a LPSS facility is a second option, we propose an SPSS facility as a first option. (author)

  18. A comparison between short pulse spallation source and long pulse spallation source

    International Nuclear Information System (INIS)

    Aizawa, Kazuya; Watanabe, Noboru; Suzuki, Jun-ichi; Niimura, Nobuo; Morii, Yukio; Katano, Susumu; Osakabe, Toyotaka; Teshigawara, Makoto; Mezei, F.

    1997-01-01

    The performance for a 5 MW short pulse spallation source (SPSS) and a 4.5 MW long pulse spallation source (LPSS) in a JAERI program which is based on the availability of a 1.5 GeV superconducting linac with a 30 mA peak current for both proton and H - beams is discussed. We have examined the superiority of SPSS to LPSS. While a LPSS facility is a second option, we propose an SPSS facility as a first option. (author)

  19. Results from the TARC experiment: spallation neutron phenomenology in lead and neutron-driven nuclear transmutation by adiabatic resonance crossing.

    CERN Document Server

    Abánades, A; Andriamonje, Samuel A; Angelopoulos, Angelos; Apostolakis, Alcibiades J; Arnould, H; Belle, E; Bompas, C A; Brozzi, Delecurgo; Bueno, J; Buono, S; Carminati, F; Casagrande, Federico; Cennini, P; Collar, J I; Cerro, E; Del Moral, R; Díez, S; Dumps, Ludwig; Eleftheriadis, C; Embid, M; Fernández, R; Gálvez, J; García, J; Gelès, C; Giorni, A; González, E; González, O; Goulas, I; Heuer, R D; Hussonnois, M; Kadi, Y; Karaiskos, P; Kitis, G; Klapisch, Robert; Kokkas, P; Lacoste, V; Le Naour, C; Lèpez, C; Loiseaux, J M; Martínez-Val, J M; Méplan, O; Nifenecker, H; Oropesa, J; Papadopoulos, I M; Pavlopoulos, P; Pérez-Enciso, E; Pérez-Navarro, A; Perlado, M; Placci, A; Poza, M; Revol, Jean Pierre Charles; Rubbia, Carlo; Rubio, J A; Sakelliou, L; Saldaña, F; Savvidis, E; Schussler, F; Sirvent, C; Tamarit, J; Trubert, D; Tzima, A; Viano, J B; Vieira, S L; Vlachoudis, V; Zioutas, Konstantin; CERN. Geneva. SPS and LEP Division

    2000-01-01

    The results of the TARC experiment are summarized herewith, whose main purpose is to demonstrate the possibility of using Adiabatic Resonance Crossing (ARC) to destroy efficiently Long-Lived Fission Fragments (LLFFs) in accelerator-driven systems and to validate a new simulation developed in the framework of the Energy Amplifier programme. An experimental set-up was installed in a CERN PS proton beam line to study how neutrons, produced by spallation at relatively high energy (En * 1 MeV), slow down quasi adiabatically, with almost flat isolethargic energy distribution and reach the capture resonance energy of an element to be transmuted where they will have a high probability of being captured. Precision measurements of energy and space distributions of spallation neutrons (using 2.5 GeV/c and 3.5 GeV/c protons) slowing down in a 3.3 m x 3.3 m x 3 m lead volume and of neutron capture rates on LLFFs 99Tc, 129I, and several other elements were performed. An appropriate formalism and appropriate computational t...

  20. VESPA: The vibrational spectrometer for the European Spallation Source

    Energy Technology Data Exchange (ETDEWEB)

    Fedrigo, Anna, E-mail: anna.fedrigo@nbi.ku.dk [Niels Bohr Institute, University of Copenhagen, 2100 Copenhagen Ø (Denmark); Istituto dei Sistemi Complessi, Consiglio Nazionale delle Ricerche, 50019 Sesto Fiorentino (Italy); European Spallation Source ESS AB, SE-221 00 Lund (Sweden); Colognesi, Daniele; Grazzi, Francesco; Zoppi, Marco [Istituto dei Sistemi Complessi, Consiglio Nazionale delle Ricerche, 50019 Sesto Fiorentino (Italy); Bertelsen, Mads; Strobl, Markus [Niels Bohr Institute, University of Copenhagen, 2100 Copenhagen Ø (Denmark); European Spallation Source ESS AB, SE-221 00 Lund (Sweden); Hartl, Monika; Deen, Pascale P. [European Spallation Source ESS AB, SE-221 00 Lund (Sweden); Lefmann, Kim [Niels Bohr Institute, University of Copenhagen, 2100 Copenhagen Ø (Denmark)

    2016-06-15

    VESPA, Vibrational Excitation Spectrometer with Pyrolytic-graphite Analysers, aims to probe molecular excitations via inelastic neutron scattering. It is a thermal high resolution inverted geometry time-of-flight instrument designed to maximise the use of the long pulse of the European Spallation Source. The wavelength frame multiplication technique was applied to provide simultaneously a broad dynamic range (about 0-500 meV) while a system of optical blind choppers allows to trade flux for energy resolution. Thanks to its high flux, VESPA will allow the investigation of dynamical and in situ experiments in physical chemistry. Here we describe the design parameters and the corresponding McStas simulations.

  1. SEE cross section calibration and application to quasi-monoenergetic and spallation facilities

    Directory of Open Access Journals (Sweden)

    Alía Rubén García

    2017-01-01

    Full Text Available We describe an approach to calibrate SEE-based detectors in monoenergetic fields and apply the resulting semi-empiric responses to more general mixed-field cases in which a broad variety of particle species and energy spectra are involved. The calibration of the response functions is based both on experimental proton and neutron data and considerations derived from Monte Carlo simulations using the FLUKA code. The application environments include the quasi-monoenergetic neutrons at RCNP, the atmospheric-like VESUVIO spallation spectrum and the CHARM high-energy accelerator test facility.

  2. CLEAR: Prospects for a low threshold neutrino experiment at the Spallation Neutron Source

    International Nuclear Information System (INIS)

    Scholberg, Kate

    2008-01-01

    A low-threshold neutrino scattering experiment at a high intensity stopped-pion neutrino source has the potential to measure coherent neutral current neutrino-nucleus elastic scattering. A promising prospect for the measurement of this process is a proposed noble-liquid-based experiment, dubbed CLEAR (Coherent Low Energy A (Nuclear) Recoils), at the Spallation Neutron Source. This poster will describe the CLEAR proposal and its physics reach.

  3. New spallation neutron sources, their performance and applications

    International Nuclear Information System (INIS)

    1985-01-01

    Pulsed spallation sources now operating in the world are at the KEK Laboratory in Japan (the KENS source), at Los Alamos National Laboratory (WNR) and at Argonne National Laboratory (IPNS), both the latter being in the US. The Intense Pulsed Neutron Source (IPNS) is currently the world's most intense source with a peak neutron flux of 4 x 10 14 n cm -2 s -1 at a repetition rate of 30 Hz, and globally producing approx. 1.5 x 10 15 n/sec. Present pulsed sources are still relatively weak compared to their potential. In 1985 the Rutherford Spallation Neutron Source will come on line, and eventually be approx. 30 more intense than the present IPNS. Later, in 1986 the WNR/PSR option at Los Alamos will make that facility of comparable intensity, while a subcritical fission booster at IPNS will keep IPNS competitive. These new sources will expand the applications of pulsed neutrons but are still based on accelerators built for other scientific purposes, usually nuclear or high-energy physics. Accelerator physicists are now designing machines expressly for spallation neutron research, and the proton currents attainable appear in the milliamps. (IPNS now runs at 0.5 GeV and 14 μA). Such design teams are at the KFA Laboratory Julich, Argonne National Laboratory and KEK. Characteristics, particularly the different time structure of the pulses, of these new sources will be discussed. Such machines will be expensive and require national, if not international, collaboration across a wide spectrum of scientific disciplines. The new opportunities for neutron research will, of course, be dramatic with these new sources

  4. Breakup reactions at intermediate and high energy

    International Nuclear Information System (INIS)

    Shotter, A.C.; Bice, A.N.

    1981-01-01

    Having considered some general aspects of peripheral break-up reactions involving heavy ions for the incident energy range 10-2000 MeV/A, specific experiments carried out at Berkeley in 1980 in the energy range 10-20 MeV/A are discussed. These indicate that sequential break-up processes from non-sequential inelastic processes both play significant roles in the mechanism. (UK)

  5. 2. International workshop on spallation materials technology

    International Nuclear Information System (INIS)

    Carsughi, F.; Mansur, L.K.; Sommer, W.F.; Ullmaier, H.

    1997-11-01

    This document contains 25 papers consisting an abstract prepared by the authors, followed by copies of the presentation viewgraphs used by speakers. The topics were: Target options for SINQ; Overview of the NSNS target system; ISIS target and moderator materials; Trispal project; JHF N-ARENA; Design, load conditions and manufacturing aspect of the ESS MERCURY TARGET unit; Radiation damage simulatiion to measure recoil spectra distribution; Radiation damage calculation to spallation neutron source materials; Hadron-induced neutron production in Pb and U targets from 1-5 GeV; Proton beam effects on W rods, surface cooled by water; Corrosion and fatigue behavior of metals and alloys in high radiation fields; compability of materials with mercury for NSNS target system; Research activities at PSI on structural materials for spallation neutron source; The accelerator production of tritium materials reserach program and Los Alamos National Laboratory; Experimental program on irradiation effects in structural materials of the Trispal project; First pulsed power materials test at Livermore; Plan of thermal shock fracture test at JAERI; Is there a hydrogen problem in target materials in high-power spatllation source?; Materials consideration for the NSNS target; Materials durability issures in spallation neutron source applications; Post-irradiation investigations at the FZJ; Microstructure and hardening of steels containing high helium concentrations; Tensile properties and microstructure of the F82H ferritic-martensitic steel after irradiation in the PIREX facility

  6. Design of an experimental device dedicated to the measurement of spallation reactions; Mise au point d'un dispositif experimental pour des mesures exclusives des reactions de spallation

    Energy Technology Data Exchange (ETDEWEB)

    Lafriakh, A

    2005-12-15

    Spallation mechanisms are not yet completely understood, especially because of the difficulty of experimentally disentangling the effects of the different steps of the reaction. In order to understand these mechanisms, we have developed a new experimental device able to perform inclusive measurements. We propose a detection system based on a combination of ionization chambers and proportional counters and on a wall of plastic scintillators to measure light charged particles. In particular the detection of light charged particles is described in detail. In order to validate our device, we have compared our preliminary results obtained on the Fe{sup 56} + p system at 1 GeV/u with inclusive measurements previously obtained at the FRS spectrometer of the GSI facility. A comparison of charge differential cross section shows reasonable agreement. However, our new device allowed extension of those measurements down to Z = 1 and Z = 2. These cross sections are important for material damage studies. Taking into account our error brackets, the evolution of mean longitudinal velocities with respect to residue masses is comparable to that obtained at the FRS. These first results, although preliminary, allow us to validate our experimental device. It is now possible to exploit the strong points of our exclusive measurements, namely correlations between different measured observables. Finally, experimental problems encountered will be taken into account in the future experimental programs, in order to ensure the best measurements conditions.

  7. Benchmarking shielding simulations for an accelerator-driven spallation neutron source

    Directory of Open Access Journals (Sweden)

    Nataliia Cherkashyna

    2015-08-01

    Full Text Available The shielding at an accelerator-driven spallation neutron facility plays a critical role in the performance of the neutron scattering instruments, the overall safety, and the total cost of the facility. Accurate simulation of shielding components is thus key for the design of upcoming facilities, such as the European Spallation Source (ESS, currently in construction in Lund, Sweden. In this paper, we present a comparative study between the measured and the simulated neutron background at the Swiss Spallation Neutron Source (SINQ, at the Paul Scherrer Institute (PSI, Villigen, Switzerland. The measurements were carried out at several positions along the SINQ monolith wall with the neutron dosimeter WENDI-2, which has a well-characterized response up to 5 GeV. The simulations were performed using the Monte-Carlo radiation transport code geant4, and include a complete transport from the proton beam to the measurement locations in a single calculation. An agreement between measurements and simulations is about a factor of 2 for the points where the measured radiation dose is above the background level, which is a satisfactory result for such simulations spanning many energy regimes, different physics processes and transport through several meters of shielding materials. The neutrons contributing to the radiation field emanating from the monolith were confirmed to originate from neutrons with energies above 1 MeV in the target region. The current work validates geant4 as being well suited for deep-shielding calculations at accelerator-based spallation sources. We also extrapolate what the simulated flux levels might imply for short (several tens of meters instruments at ESS.

  8. Total cross-sections for reactions of high energy particles (including elastic, topological, inclusive and exclusive reactions). Subvol. b

    International Nuclear Information System (INIS)

    Schopper, H.; Moorhead, W.G.; Morrison, D.R.O.

    1988-01-01

    The aim of this report is to present a compilation of cross-sections (i.e. reaction rates) of elementary particles at high energy. The data are presented in the form of tables, plots and some fits, which should be easy for the reader to use and may enable him to estimate cross-sections for presently unmeasured energies. We have analyzed all the data published in the major Journals and Reviews for momenta of the incoming particles larger than ≅ 50 MeV/c, since the early days of elementary particle physics and, for each reaction, we have selected the best cross-section data available. We have restricted our attention to integrated cross-sections, such as total cross-sections, exclusive and inclusive cross-sections etc., at various incident beam energies. We have disregarded data affected by geometrical and/or kinematical cuts which would make them not directly comparable to other data at different energies. Also, in the case of exclusive reactions, we have left out data where not all of the particles in the final state were unambiguously identified. This work contains reactions induced by neutrinos, gammas, charged pions, kaons, nucleons, antinucleons and hyperons. (orig./HSI)

  9. Measurement and analysis of turbulent liquid metal flow in a high-power spallation neutron source-EURISOL

    CERN Document Server

    Samec, K; Blumenfeld, L; Kharoua, C; Dementjevs, S; Milenkovic, R Z

    2011-01-01

    The European Isotope Separation On-Line (EURISOL) design study completed in 2009 examined means of producing exotic nuclei for fundamental research. One of the critical components identified in the study was a high-power neutron spallation source in which a target material is impacted by a proton beam producing neutrons by a process known as spallation. Due to the high heat power deposition, liquid metal, in this case mercury, is the only viable choice as target material. Complex issues arise from the use of liquid metal. It is characterised by an unusually low Prandtl number and a higher thermal expansivity than conventional fluids. The turbulence structure in LM is thereby affected and still an object of intense research, hampered in part by measurement difficulties. The use of Computational Fluid Dynamics (CFD) allowed a satisfactory design for the neutron source to be found rapidly with little iteration. However it was feared that the development of the boundary layer and associated turbulence would not b...

  10. Study of measurement method of tritium induced in concrete of high-energy proton accelerator facilities

    International Nuclear Information System (INIS)

    Ohtsuka, N.; Ishihama, S.; Kunifuda, T.; Hayasaka, N.; Miura, T.

    2001-01-01

    Various long-loved radionuclides, 3 H, 7 Be, 22 Na, 51 Cr, 54 Mn, 56 Co, 57 Co, 60 Co, 134 Cs, 152 Eu and 154 Eu, have been produced in the shielding concrete of high energy proton accelerator facility through both nuclear spallation reactions and thermal neutron capture reactions of concrete elements, during machine operation. Tritium is the most important nuclide from the radiation protection. There were, however, few measurements of tritium concentration induced in the shielding concrete. In this study, the conditions of measurement method of tritium concentration induced in shielding concrete have been investigated using the activated shielding concrete of the 12 GeV proton beam-line tunnel at KEK and the standard rock (JG-1) irradiated of thermal neutron at the reactor. And the depth profiles of tritium induced in the shielding concrete of slow extracted proton beam line at KEK were determined using this method. (author)

  11. Production of residual nuclides by proton-induced reactions on target W at the energy of 72 MeV

    Energy Technology Data Exchange (ETDEWEB)

    Miah, Moazzem Hossain [Univ. of Chittagong, Dept. of Physics, Chittagong (Bangladesh); Kuhnhenn, Jochen; Herpers, Ulrich [Univ. of Cologne, Dept. of Nuclear Chemistry, Cologne (Germany); Michel, Rolf [University of Hannover, Centre for Radiation Protection and Radioecology (Germany); Kubik, Peter [Paul Scherrer Inst., c/o Institute for Particle Physics, ETH Hoenggerberg, Zuerich (Switzerland)

    2002-08-01

    Investigations of cross-sections for residual nuclide production on the target element W by proton-induced reactions were performed by irradiating the target with 72 MeV protons using the cyclotron facilities at Paul-Scherrer Institute, Zurich, Switzerland. Residual nuclides were measured by gamma-spectrometry of HpGe detectors calibrated with standard gamma sources. The measured data contains 104 individual cross-sections for 20 identified nuclides in the proton energies between 52.5 - 68.9 MeV. These nuclear data is important in the study of spallation neutron source and in accelerator driven technologies such as waste transmutation and energy amplification. The present data are compared with the shape of the excitation functions of earlier only one measurement at higher energies and they are in good agreement to each other. (author)

  12. Probing the nuclear symmetry energy at high densities with nuclear reactions

    Science.gov (United States)

    Leifels, Y.

    2017-11-01

    The nuclear equation of state is a topic of highest current interest in nuclear structure and reactions as well as in astrophysics. The symmetry energy is the part of the equation of state which is connected to the asymmetry in the neutron/proton content. During recent years a multitude of experimental and theoretical efforts on different fields have been undertaken to constraint its density dependence at low densities but also above saturation density (ρ_0=0.16 fm ^{-3} . Conventionally the symmetry energy is described by its magnitude S_v and the slope parameter L , both at saturation density. Values of L = 44 -66MeV and S_v=31 -33MeV have been deduced in recent compilations of nuclear structure, heavy-ion reaction and astrophysics data. Apart from astrophysical data on mass and radii of neutron stars, heavy-ion reactions at incident energies of several 100MeV are the only means do access the high density behaviour of the symmetry energy. In particular, meson production and collective flows upto about 1 AGeV are predicted to be sensitive to the slope of the symmetry energy as a function of density. From the measurement of elliptic flow of neutrons with respect to charged particles at GSI, a more stringent constraint for the slope of the symmetry energy at supra-saturation densities has been deduced. Future options to reach even higher densities will be discussed.

  13. Triple ion-beam studies of radiation damage effects in a 316LN austenitic alloy for a high power spallation neutron source

    International Nuclear Information System (INIS)

    Lee, E.H.; Rao, G.R.; Hunn, J.D.; Rice, P.M.; Lewis, M.B.; Cook, S.W.; Farrell, K.; Mansur, L.K.

    1997-09-01

    Austenitic 316LN alloy was ion-irradiated using the unique Triple Ion Beam Facility (TIF) at ORNL to investigate radiation damage effects relevant to spallation neutron sources. The TIF was used to simulate significant features of GeV proton irradiation effects in spallation neutron source target materials by producing displacement damage while simultaneously injecting helium and hydrogen at appropriately high gas/dpa ratios. Irradiations were carried out at 80, 200, and 350 C using 3.5 MeV Fe ++ , 360 keV He + , and 180 keV H + to accumulate 50 dpa by Fe, 10,000 appm of He, and 50,000 appm of H. Irradiations were also carried out at 200 C in single and dual ion beam modes. The specific ion energies were chosen to maximize the damage and the gas accumulation at a depth of ∼ 1 microm. Variations in microstructure and hardness of irradiated specimens were studied using transmission electron microscopy (TEM) and a nanoindentation technique, respectively. TEM investigation yielded varying damage defect microstructures, comprising black dots, faulted and unfaulted loops, and a high number density of fine bubbles (typically less than 1 nm in diameter). With increasing temperature, faulted loops had a tendency to unfault, and bubble microstructure changed from a bimodal size distribution to a unimodal distribution. Triple ion irradiations at the three temperatures resulted in similar increases in hardness of approximately a factor of two. Individually, Fe and He ions resulted in a similar magnitude of hardness increase, whereas H ions showed only a very small effect. The present study has yielded microstructural information relevant to spallation neutron source conditions and indicates that the most important concern may be radiation induced hardening and associated ductility loss

  14. Triple Ion-Beam Studies of Radiation Damage Effects in a 316LN Austenitic Alloy for a High Power Spallation Neutron Source

    International Nuclear Information System (INIS)

    Lee, E.H.

    2001-01-01

    Austenitic 316LN alloy was ion-irradiated using the unique Triple Ion Beam Facility (TIF) at ORNL to investigate radiation damage effects relevant to spallation neutron sources. The TIF was used to simulate significant features of GeV proton irradiation effects in spallation neutron source target materials by producing displacement damage while simultaneously injecting helium and hydrogen at appropriately high gas/dpa ratios. Irradiations were carried out at 80, 200, and 350 C using 3.5 MeV Fe 2 , 360 keV He + , and 180 keV H + to accumulate 50 dpa by Fe, 10,000 appm of He, and 50,000 appm of H. Irradiations were also carried out at 200 C in single and dual ion beam modes. The specific ion energies were chosen to maximize the damage and the gas accumulation at a depth of ∼ 1 microm. Variations in microstructure and hardness of irradiated specimens were studied using transmission electron microscopy (TEM) and a nanoindentation technique, respectively. TEM investigation yielded varying damage defect microstructures, comprising black dots, faulted and unfaulted loops, and a high number density of fine bubbles (typically less than 1 nm in diameter). With increasing temperature, faulted loops had a tendency to unfault, and bubble microstructure changed from a bimodal size distribution to a unimodal distribution. Triple ion irradiations at the three temperatures resulted in similar increases in hardness of approximately a factor of two. Individually, Fe and He ions resulted in a similar magnitude of hardness increase, whereas H ions showed only a very small effect. The present study has yielded microstructural information relevant to spallation neutron source conditions and indicates that the most important concern may be radiation induced hardening and associated ductility loss

  15. Neutronic performance issues for the Spallation Neutron Source moderators

    International Nuclear Information System (INIS)

    Iverson, E.B.; Murphy, B.D.

    2001-01-01

    We continue to develop the neutronic models of the Spallation Neutron Source target station and moderators in order to better predict the neutronic performance of the system as a whole and in order to better optimize that performance. While we are not able to say that every model change leads to more intense neutron beams being predicted, we do feel that such changes are advantageous in either performance or in the accuracy of the prediction of performance. We have computationally and experimentally studied the neutronics of hydrogen-water composite moderators such as are proposed for the SNS Project. In performing these studies, we find that the composite moderator, at least in the configuration we have examined, does not provide performance characteristics desirable for the instruments proposed and being designed for this neutron scattering facility. The pulse width as a function of energy is significantly broader than for other moderators, limiting attainable resolution-bandwidth combinations. Furthermore, there is reason to expect that higher-energy (0.1-1 eV) applications will be significantly impacted by bimodal pulse shapes requiring enormous effort to parameterize. As a result of these studies, we have changed the SNS design, and will not use a composite moderator at this time. We have analyzed the depletion of a gadolinium poison plate in a hydrogen moderator at the Spallation Neutron Source, and found that conventional poison thicknesses will be completely unable to last the desired component lifetime of three operational years. A poison plate 300-600 μm thick will survive for the required length of time, but will somewhat degrade the intensity (by as much as 15% depending on neutron energy) and the consistency of the neutron source performance. Our results should scale fairly easily to other moderators on this or any other spallation source. While depletion will be important for all highly-absorbing materials in high-flux regions, we feel it likely that

  16. Beam Instrumentation for the Spallation Neutron Source Ring

    International Nuclear Information System (INIS)

    Witkover, R. L.; Cameron, P. R.; Shea, T. J.; Connolly, R. C.; Kesselman, M.

    1999-01-01

    The Spallation Neutron Source (SNS) will be constructed by a multi-laboratory collaboration with BNL responsible for the transfer lines and ring. The 1 MW beam power necessitates careful monitoring to minimize un-controlled loss. This high beam power will influence the design of the monitors in the high energy beam transport line (HEBT) from linac to ring, in the ring, and in the ring-to-target transfer line (RTBT). The ring instrumentation must cover a 3-decade range of beam intensity during accumulation. Beam loss monitoring will be especially critical since un-controlled beam loss must be kept below 10 -4 . A Beam-In-Gap (BIG) monitor is being designed to assure out-of-bucket beam will not be lost in the ring

  17. Safety analysis and lay-out aspects of shieldings against particle radiation at the example of spallation facilities in the megawatt range

    International Nuclear Information System (INIS)

    Hanslik, R.

    2006-08-01

    This paper discusses the shielding of particle radiation from high current accelerators, spallation neutron sources and so called ADS-facilities (Accelerator Driven Systems). ADS-facilities are expected to gain importance in the future for transmutation of long-lived isotopes from fission reactors as well as for energy production. In this paper physical properties of the radiation as well as safety relevant requirements and corresponding shielding concepts are discussed. New concepts for the layout and design of such shielding are presented. Focal point of this work will be the fundamental difference between conventional fission reactor shielding and the safety relevant issues of shielding from high-energy radiation. Key point of this paper is the safety assessment of shielding issues of high current accelerators, spallation targets and ADS-blanket systems as well as neutron scattering instruments at spallation neutron sources. Safety relevant shielding requirements are presented and discussed. For the layout and design of the shielding for spallation sources computer base calculations methods are used. A discussion and comparison of the most important methods like semi-empirical, deterministic and stochastic codes are presented. Another key point within the presented paper is the discussion of shielding materials and their shielding efficiency concerning different types of radiation. The use of recycling material, as a cost efficient solution, is discussed. Based on the conducted analysis, flowcharts for a systematic layout and design of adequate shielding for targets and accelerators have been developed and are discussed in this paper. By use of these flowcharts layout and engineering design of future ADS-facilities can be performed. (orig.)

  18. The 3rd Nordic meeting on high energy reactions in nuclei

    International Nuclear Information System (INIS)

    Green, A.M.; Kullander, S.

    Abstracts of the 31 lectures given at the meeting are presented. Major emphasis was placed on the nucleon-nucleon and nucleon-antinucleon interaction in bound and unbound systems. Four of the ten sessions were devoted to this subject. Two sessions contained lecture and seminars on 'Isobars in nuclei', two were devoted to hadron-nucleus reactions, one to high-energy heavy-ion reactions and one to new developments of experimental tools. This latter session had two talks, one about channeling with GeV particles and the other about the planned low-energy antiproton facility LEAR at CERN. Talks of more general character were 'The experimental programme at the CERN SC', 'Accelerator produced nuclear fuel' and 'The upsilons, a new family of quark-antiquark bound state'. (JIW)

  19. Materials considerations for the National Spallation Neutron Source target

    International Nuclear Information System (INIS)

    Mansur, L.K.; DiStefano, J.R.; Farrell, K.; Lee, E.H.; Pawel, S.J.; Wechsler, M.S.

    1997-08-01

    The National Spallation Neutron Source (NSNS), in which neutrons are generated by bombarding a liquid mercury target with 1 GeV protons, will place extraordinary demands on materials performance. The target structural material will operate in an aggressive environment, subject to intense fluxes of high energy protons, neutrons, and other particles, while exposed to liquid mercury and to water. Components that require special consideration include the Hg liquid target container and protective shroud, beam windows, support structures, moderator containers, and beam tubes. In response to these demands a materials R and D program has been developed for the NSNS that includes: selection of materials; calculations of radiation damage; irradiations, post irradiation testing, and characterization; compatibility testing and characterization; design and implementation of a plan for monitoring of materials performance in service; and materials engineering and technical support to the project. Irradiations are being carried out in actual and simulated spallation environments. Compatibility experiments in Hg are underway to ascertain whether the phenomena of liquid metal embrittlement and temperature gradient mass transfer will be significant. Results available to date are assessed in terms of the design and operational performance of the facility

  20. Experimental studies of spallation on thin target; Etudes experimentales de la spallation en cible mince

    Energy Technology Data Exchange (ETDEWEB)

    Borne, F.; Crespin, S.; Drake, D.; Frehaut, J.; Ledoux, X.; Lochard, J.P.; Martinez, E.; Patin, Y.; Petibon, E.; Pras, Ph. [CEA/DAM-Ile de France, Dept. de Physique Theorique et Appliquee, DPTA, 91 - Bruyeres-Le-Chatel (France); Boudard, A.; Legrain, R.; Leray, S.; Terrien, Y. [CEA/Saclay, Dept. d' Astrophysique, de la Physique des Particules, de la Physique Nucleaire et de l' Instrumentation Associee, DAPNIA, 91 - Gif-sur-Yvette (France); Bouyer, P.; Brochard, F.; Duchazeaubeneix, J.C.; Durand, J.M.; Meigo, S.I.; Milleret, G.; Thun, J.; Whittal, D.M.; Wlazlo, W. [Laboratoire National Saturne - Centre d' Etudes Nucleaires de Saclay, 91 - Gif-sur-Yvette (France); Lebrun, C.; Lecolley, J.F.; Lecolley, F.R.; Lefebvres, F.; Louvel, M.; Varignon, C. [Caen Univ., Lab. de Physique Corpusculaire, 14 (France); Menard, S. [Institut de Physique Nucleaire, IN2P3/CNRS, 91 - Orsay (France); Stugge, L. [Institut de Recherches Subatomiques, IReS, 67 - Strasbourg (France); Hanappe, F. [IIM, Bruxelles (Belgium)

    2000-07-01

    Angular distribution of spallation neutrons induced by protons (0.8, 1.2 and 1.6 GeV) and deuterons (0.8 and 1.6 GeV) beams on various thin targets have been measured at SATURNE (CEA Saclay/France) with two complementary experimental techniques: the time-of-flight measurement with tagged incident protons for low energy neutrons (2-400 MeV) and the use of a hydrogen converter associated are analysed, interpreted and finally compared with theoretical previsions of simulation codes using the TIERCE system including the intranuclear cascade codes of BERTINI and CUGNON. (authors)

  1. Thermal hydraulic studies of lead–bismuth eutectic spallation target of CIADS

    Energy Technology Data Exchange (ETDEWEB)

    Chen, Kang [Institute of Modern Physics, Chinese Academy of Sciences, 509 Nanchang Rd., Lanzhou, Gansu 730000 (China); University of Chinese Academy of Sciences, 19 A Yuquan Rd, Shijingshan District, Beijing 100049 (China); Yang, Yongwei, E-mail: yangyongwei@impcas.ac.cn [Institute of Modern Physics, Chinese Academy of Sciences, 509 Nanchang Rd., Lanzhou, Gansu 730000 (China); Fan, Deliang; Gao, Yucui [Institute of Modern Physics, Chinese Academy of Sciences, 509 Nanchang Rd., Lanzhou, Gansu 730000 (China)

    2016-08-15

    Highlights: • A 3-D fluid-solid coupling thermal-hydraulic analysis is made for the LBE target. • The reactor and the spallation target is coupled in thermal process. • The heat transfer between the inlet and outlet of the spallation target is taken into account. - Abstract: For the China Initiative Accelerator Driven System (CIADS), it includes three sub-systems: accelerator, spallation target, and sub-critical reactor. The sub-system of spallation target is an important component of the CIADS, which is coupled with the other two sub-systems. The proton beam from the accelerator with an energy of 250 MeV and a current intensity of 2 mA reacts with the nuclei of the lead–bismuth eutectic (LBE), approximately 0.5 MW of heat is deposited in the target zone, which must be removed by circulating the LBE. To reach the goal, we carried out the study by using the Computational Fluid Dynamics (CFD) software FLUENT, to study the flow patterns and temperature distribution in the target zone. For these simulations, the heat transferred from the sub-critical reactor was taken into account. The results indicated that the heat deposited in the target zone can be removed safely.

  2. Neutron moderators for the European Spallation Source

    DEFF Research Database (Denmark)

    Klinkby, Esben Bryndt; Zanini, L.; Batkov, K.

    The design of the neutron moderators for the European Spallation Source, intended to be installed at the start of operations of the facility in 2019 has now been finalized and the moderators are being fabricated. Among the driving principles in the design have been flexibility for instruments...... to have access to cold and thermal neutrons with highest possible source brightness. Different design and configuration options were evaluated. The final configuration accepted for construction foresees two moderators with identical para-hydrogen (so-called "butterfly") shape, but different heights......, placed above and below the spallation target. Both moderators are able to serve the full 2 x 120° beam extraction sectors of instrument suite. The top, 3-cm tall moderator, has both high thermal and high cold brightness, more than by a factor of 2.5 compared to the previous design of the Technical Design...

  3. Strain rate effects for spallation of concrete

    Science.gov (United States)

    Häussler-Combe, Ulrich; Panteki, Evmorfia; Kühn, Tino

    2015-09-01

    Appropriate triaxial constitutive laws are the key for a realistic simulation of high speed dynamics of concrete. The strain rate effect is still an open issue within this context. In particular the question whether it is a material property - which can be covered by rate dependent stress strain relations - or mainly an effect of inertia is still under discussion. Experimental and theoretical investigations of spallation of concrete specimen in a Hopkinson Bar setup may bring some evidence into this question. For this purpose the paper describes the VERD model, a newly developed constitutive law for concrete based on a damage approach with included strain rate effects [1]. In contrast to other approaches the dynamic strength increase is not directly coupled to strain rate values but related to physical mechanisms like the retarded movement of water in capillary systems and delayed microcracking. The constitutive law is fully triaxial and implemented into explicit finite element codes for the investigation of a wide range of concrete structures exposed to impact and explosions. The current setup models spallation experiments with concrete specimen [2]. The results of such experiments are mainly related to the dynamic tensile strength and the crack energy of concrete which may be derived from, e.g., the velocity of spalled concrete fragments. The experimental results are compared to the VERD model and two further constitutive laws implemented in LS-Dyna. The results indicate that both viscosity and retarded damage are required for a realistic description of the material behaviour of concrete exposed to high strain effects [3].

  4. Strain rate effects for spallation of concrete

    Directory of Open Access Journals (Sweden)

    Häussler-Combe Ulrich

    2015-01-01

    Full Text Available Appropriate triaxial constitutive laws are the key for a realistic simulation of high speed dynamics of concrete. The strain rate effect is still an open issue within this context. In particular the question whether it is a material property – which can be covered by rate dependent stress strain relations – or mainly an effect of inertia is still under discussion. Experimental and theoretical investigations of spallation of concrete specimen in a Hopkinson Bar setup may bring some evidence into this question. For this purpose the paper describes the VERD model, a newly developed constitutive law for concrete based on a damage approach with included strain rate effects [1]. In contrast to other approaches the dynamic strength increase is not directly coupled to strain rate values but related to physical mechanisms like the retarded movement of water in capillary systems and delayed microcracking. The constitutive law is fully triaxial and implemented into explicit finite element codes for the investigation of a wide range of concrete structures exposed to impact and explosions. The current setup models spallation experiments with concrete specimen [2]. The results of such experiments are mainly related to the dynamic tensile strength and the crack energy of concrete which may be derived from, e.g., the velocity of spalled concrete fragments. The experimental results are compared to the VERD model and two further constitutive laws implemented in LS-Dyna. The results indicate that both viscosity and retarded damage are required for a realistic description of the material behaviour of concrete exposed to high strain effects [3].

  5. X-ray quantitative analysis on spallation response in high purity copper under sweeping detonation

    Energy Technology Data Exchange (ETDEWEB)

    Yang, Yang, E-mail: yangyanggroup@163.com [School of Material Science and Engineering, Central South University, Changsha 410083 (China); Institute of Fluid Physics, China Academy of Engineering Physics, Mianyang 621900 (China); National Key Laboratory of Explosion Science and Technology, Beijing Institute of Technology, Beijing 100081 (China); Key Laboratory of Nonferrous Metals Material Science and Engineering of Ministry of Education, Central South University, Changsha 410083 (China); Chen, Jixiong; Peng, Zhiqiang [School of Material Science and Engineering, Central South University, Changsha 410083 (China); Guo, Zhaoliang; Tang, Tiegang; Hu, Haibo [Institute of Fluid Physics, China Academy of Engineering Physics, Mianyang 621900 (China); Hu, Yanan [Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201800 (China)

    2016-06-14

    The 3-D quantitative investigation of spall behavior in high purity copper plants with different heat treatment histories was characterized using X-ray computer tomography (XRCT). The effect of shock stress and grain size on the spatial distribution and morphology of incipient spall samples were discussed. The results revealed that, in samples with similar microstructure, the ranges of void distribution decrease with the increasing of shock stress. The characteristic parameters (such as mean elongation, mean flatness and mean sphericity of voids) determined using XRCT herein as a function of shock stress and grain size. The quantitative analyses of spallation datasets render functional relationships between the microscopic parameters (like volume, frequency) of spallation voids and the microstructure. The XRCT observations show that voids are prone to coalescence in thermo-mechanical treatments (TMT) sample, while the final maximum and mean volume of void were smaller than that of annealed sample. This is due to the smaller grain size of TMT sample, which means more nucleation sites of voids, this made the voids get closer and easier to coalescence, and flat voids formed ultimately.

  6. Neutron scattering instrumentation for biology at spallation neutron sources

    Energy Technology Data Exchange (ETDEWEB)

    Pynn, R. [Los Alamos National Laboratory, NM (United States)

    1994-12-31

    Conventional wisdom holds that since biological entities are large, they must be studied with cold neutrons, a domain in which reactor sources of neutrons are often supposed to be pre-eminent. In fact, the current generation of pulsed spallation neutron sources, such as LANSCE at Los Alamos and ISIS in the United Kingdom, has demonstrated a capability for small angle scattering (SANS) - a typical cold- neutron application - that was not anticipated five years ago. Although no one has yet built a Laue diffractometer at a pulsed spallation source, calculations show that such an instrument would provide an exceptional capability for protein crystallography at one of the existing high-power spoliation sources. Even more exciting is the prospect of installing such spectrometers either at a next-generation, short-pulse spallation source or at a long-pulse spallation source. A recent Los Alamos study has shown that a one-megawatt, short-pulse source, which is an order of magnitude more powerful than LANSCE, could be built with today`s technology. In Europe, a preconceptual design study for a five-megawatt source is under way. Although such short-pulse sources are likely to be the wave of the future, they may not be necessary for some applications - such as Laue diffraction - which can be performed very well at a long-pulse spoliation source. Recently, it has been argued by Mezei that a facility that combines a short-pulse spallation source similar to LANSCE, with a one-megawatt, long-pulse spallation source would provide a cost-effective solution to the global shortage of neutrons for research. The basis for this assertion as well as the performance of some existing neutron spectrometers at short-pulse sources will be examined in this presentation.

  7. Uranium target fragmentation by intermediate and high energy 12C and 20Ne ions

    International Nuclear Information System (INIS)

    McGaughey, P.L.; Loveland, W.; Morrissey, D.J.; Aleklett, K.; Seaborg, G.T.

    1985-01-01

    Target fragment formation cross sections for nuclides with 24 12 C and 8.0 and 20.0 GeV 20 Ne with 238 U. Fragment isobaric yields were deduced from these data. The light fragment (A 12 C projectile energy of 1.0 GeV, the n-deficient fragments appear to originate primarily from a fission rather than a spallation process.) The excitation functions of the heavy fragments with 60 60, indicating that the general pattern of yields of these fragments is governed by the excitation energy deposited in the nucleus during the first step of the reaction and the geometry of the collision

  8. Bench mark spectra for high-energy neutron dosimetry

    International Nuclear Information System (INIS)

    Dierckx, R.

    1986-01-01

    To monitor radiation damage experiments, activation detectors are commonly used. The precision of the results obtained by the multiple foil analysis is largely increased by the intercalibration in bench-mark spectra. This technique is already used in dosimetry measurements for fission reactors. To produce neutron spectra similar to fusion reactor and high-energy high-intensity neutron sources (d-Li or spallation), accelerators can be used. Some possible solutions as p-Be and d-D 2 O neutron sources, useful as bench-mark spectra are described. (author)

  9. Calculated intensity of high-energy neutron beams

    International Nuclear Information System (INIS)

    Mustapha, B.; Nolen, J.A.; Back, B.B.

    2004-01-01

    The flux, energy and angular distributions of high-energy neutrons produced by in-flight spallation and fission of a 400 MeV/A 238 U beam and by the break-up of a 400 MeV/A deuteron beam are calculated. In both cases very intense secondary neutron beams are produced, peaking at zero degrees, with a relatively narrow energy spread. Such secondary neutron beams can be produced with the primary beams from the proposed rare isotope accelerator driver linac. The break-up of a 400 kW deuteron beam on a liquid-lithium target can produce a neutron flux of >10 10 neutrons/cm 2 /s at a distance of 10 m from the target

  10. High energy halogen atom reactions activated by nuclear transformations. Progress report, February 15, 1978--February 14, 1979

    International Nuclear Information System (INIS)

    Rack, E.P.

    1979-02-01

    High energy reactions of halogen atoms or ions, activated by nuclear transformations, were studied in gaseous, high pressure and condensed phase saturated and unsaturated hydrocarbons, halomethanes and other organic systems in order to better understand the mechanisms and dynamics of high energy monovalent species. The experimental and theoretical program consists of six interrelated areas: (1) the reactions of iodine with alkenes and alkynes activated by radiative neutron capture and isomeric transition in low pressure gaseous systems employing additives and rare gas moderators, high pressure and liquid systems; (2) the gas to condensed state transition in halogen high chemistry, involving bromine activated by the (n,γ) and (I.T.) processes in ethane was investigated in more detail; (3) systematics of halogen hot atom reactions. The reactions of 80 Br/sup m/, 80 Br, 82 Br/sup m/ + 82 Br, 82 Br, 128 I, 130 I, and 130 I/sup m/ + 130 I activated by radiative neutron capture or isomeric transition in hydrocarbons and halo-substituted alkanes in low pressure and high pressure gaseous systems employing additives and rare gas moderators; (4) kinetic theory applications of high energy reactions and mathematical development of caging mechanisms were developed; (5) the sterochemistry of 38 Cl substitution reactions involving diastereomeric 1,2-dichloro-1,2-difluorethane in liquid mixtures was completed, suggesting that the stereochemical course of the substitution process is controlled by the properties of the solvent molecules; and (6) the applications of high energy chemistry techniques and theory to neutron activation analysis of biological systems was continued, especially involving aluminum and vanadium trace determinations

  11. Neutrino physics at the spallation neutron source. Pt. 2

    International Nuclear Information System (INIS)

    Gabriel, T.A.; Lillie, R.A.; Bishop, B.L.; Wilczynski, J.; Zeitnitz, B.

    1981-06-01

    The shielding and detector analysis associated with a contemplated low energy (approx. equal to10 to 50 MeV) neutrino experiment at a spallation neutron source are presented and discussed. This analysis includes neutrino production and interaction rates, time dependence of the neutrino pulse, shielding considerations for neutrons coming directly from the spallation source and those which are scattered from other experimental areas, shielding considerations for galactic sources especially muons and finally detector responses to neutrino and background radiations. In general for a 1 mA (200 ns/pulse, 100 Hz), 1.1 GeV proton beam incident on a lead target surrounded by a moderator system, approximately 8 m of iron are required to reduce the background so that the event rate in the detector systems is approx. [de

  12. Hadron--hadron reactions, high multiplicity

    International Nuclear Information System (INIS)

    Diebold, R.

    1978-09-01

    A coverage of results on high energy and high multiplicity hadron reactions, charm searches and related topics, ultrahigh energy events and exotic phenomena (cosmic rays), and the nuclear effects in high energy collisions and related topics is discussed. 67 references

  13. Final stage of high energy hadron-nucleus nuclear collision reactions

    International Nuclear Information System (INIS)

    Strugal'ski, Z.; Jedrzejec, H.; Strugalska-Gola, E.; Mulas, E.

    1996-01-01

    The final or 'slow' stage of the hadron-nucleus collision reactions at high energy is considered on the basis of the collision mechanism prompted experimentally. The transmutation process of the damaged target nucleus into nucleons and stable nuclear fragments is discussed. Relations between intensities or multiplicities n p of the emitted fast protons and the mean intensities or multiplicities b > of the evaporated nucleons and nuclear fragments are presented. 14 refs

  14. High-power spallation target using a heavy liquid metal free surface flow

    International Nuclear Information System (INIS)

    Litfin, K.; Fetzer, J.R.; Batta, A.; Class, A.G.; Wetzel, Th.

    2015-01-01

    A prototype of a heavy liquid metal free surface target as proposed for the multi-purpose hybrid research reactor for high-tech applications in Mol, Belgium, has been set up and experimentally investigated at the Karlsruhe Liquid Metal Laboratory. A stable operation was demonstrated in a wide range of operating conditions and the surface shape was detected and compared with numerical pre-calculations employing Star-CD. Results show a very good agreement of experiment and numerical predictions which is an essential input for other windowless target designs like the META:LIC target for the European Spallation Source. (author)

  15. Synthesis of neutron-rich transuranic nuclei in fissile spallation targets

    OpenAIRE

    Mishustin, Igor; Malyshkin, Yury; Pshenichnov, Igor; Greiner, Walter

    2014-01-01

    A possibility of synthesizing neutron-reach super-heavy elements in spallation targets of Accelerator Driven Systems (ADS) is considered. A dedicated software called Nuclide Composition Dynamics (NuCoD) was developed to model the evolution of isotope composition in the targets during a long-time irradiation by intense proton and deuteron beams. Simulation results show that transuranic elements up to Bk-249 can be produced in multiple neutron capture reactions in macroscopic quantities. Howeve...

  16. Potential design modifications for the High Yield Lithium Injection Fusion Energy (HYLIFE) reaction chamber

    International Nuclear Information System (INIS)

    Pitts, J.H.; Hovingh, J.; Meier, W.R.; Monsler, M.J.; Powell, E.G.; Walker, P.E.

    1979-01-01

    Generation of electric power from inertial confinement fusion requires a reaction chamber. One promising type, the High Yield Lithium Injection Fusion Energy (HYLIFE) chamber, includes a falling array of liquid lithium jets. These jets act as: (1) a renewable first wall and blanket to shield metal components from x-ray and neutron exposure, (2) a tritium breeder to replace tritium burned during the fusion process, and (3) an absorber and transfer medium for fusion energy. Over 90% of the energy produced in the reaction chamber is absorbed in the lithium jet fall. Design aspects are included

  17. Experimental and Theoretical Investigations to Improve the Predictive Power of Nuclear Reaction Models in Spallation Neutron Production

    International Nuclear Information System (INIS)

    Nuenighoff, K.; Filges, D.; Goldenbaum, F.; Neef, R.D.; Nuenighoff, K.; Paul, N.; Schaal, H.; Sterzenbach, G.; Wohlmuther, M.; Enke, M.; Herbach, C.M.; Hilscher, D.; Jahnke, U.; Tishchenko, V.; Galin, J.; Letourneau, A.; Lott, B.; Peghaire, A.; Pienkowski, L.; Schroeder, U.; Toke, J.; Tietze, A.

    2002-01-01

    In order to design the target station of the European Spallation Source ESS measurements of the neutron production in possible target materials like Pb, Hg and W were performed. The aim of these measurements was to validate the simulation codes and to proof their predictive power. The NESSI experiment allows for the comparison of neutron multiplicity distributions between experiment and simulation, which is a much more sensitive method than only comparing the mean neutron multiplicities. An agreement of better than 10 % was achieved. Various target geometries with diameters up to 15 cm and lengths up to 35 cm over a range from 0.4 till 2.5 GeV incident proton energy were studied. The Monte-Carlo Simulations were performed with the HERMES, LCS, and MCNPX code system. (authors)

  18. Decommissioning and safety issues of liquid-mercury waste generated from high power spallation sources with particle accelerators

    CERN Document Server

    Chiriki, S; Odoj, R; Moormann, R; Hinssen, H. K; Bukaemskiy, A

    2009-01-01

    Large spallation sources are intended to be constructed in Europe (EURISOL nuclear physics facility and ESS-European Spallation Source). These facilities accumulate more than 20 metric tons of irradiated mercury in the target, which has to be treated as highly radioactive and chemo-toxic waste. Because solids are the only appropriate (immobile) form for this radiotoxic and toxic type of waste solidification is required for irradiated mercury. Our irradiation experimental studies on mercury waste revealed that mercury sulfide is a reasonable solid for disposal and shows larger stability in assumed accidents with water ingress in a repository compared to amalgams. For preparation of mercury sulfide a wet process is more suitable than a dry one. It is easier to perform under hot cell conditions and allows complete Hg-conversion. Embedding HgS in a cementitious matrix increases its stability.

  19. Direct reactions induced by 16O on 208Pb at high incident energy

    International Nuclear Information System (INIS)

    Mermaz, M.C.

    1978-01-01

    Direct reactions induced by 16 O mainly on 208 Pb at 20 MeV/nucleon are reviewed. The quasi-elastic transfer reaction, such as one-proton and one-neutron transfer respectively leading to 209 Bi and 209 Pb single-particle-states, is first discussed, the fragmentation of 16 O projectile on heavy targets is then envisaged. The one-nucleon transfer can be described within the framework of one-step processes using the DWBA formalism to calculate the cross sections. At high incident energy (312.6 MeV), transfer reactions involving nucleons from the deeper 1p 3/2 orbit of 16 O are kinematically favoured and well observed. At 20 MeV/A and above, a large part of the reaction cross sections seems to be due to the fragmentation of the projectile; more especially, an abrasion-ablation model have to be used in order to explain the general trend of the data (energy spectra and angular distribution)

  20. The effect of annealing and desulfurization on oxide spallation of turbine airfoil material

    International Nuclear Information System (INIS)

    Briant, C.L.; Murphy, W.H.; Schaeffer, J.C.

    1995-01-01

    In this paper the authors report a study that addresses the sulfur-induced spallation theory. Previous work has shown that a high temperature anneal in hydrogen desulfurizes nickel-base alloys and greatly improves their resistance to oxide spallation. The authors will show that such an anneal can be applied successfully to a Ni-base airfoil material. Both Auger segregation experiments and chemical analyses show that this anneal desulfurizes the material, at least in the absence of yttrium. However, the results suggest that factors other than desulfurization may be contributing to the improvement in spallation resistance produced by the anneal

  1. The Spallation Neutron Source (SNS) conceptual design shielding analysis

    International Nuclear Information System (INIS)

    Johnson, J.O.; Odano, N.; Lillie, R.A.

    1998-03-01

    The shielding design is important for the construction of an intense high-energy accelerator facility like the proposed Spallation Neutron Source (SNS) due to its impact on conventional facility design, maintenance operations, and since the cost for the radiation shielding shares a considerable part of the total facility costs. A calculational strategy utilizing coupled high energy Monte Carlo calculations and multi-dimensional discrete ordinates calculations, along with semi-empirical calculations, was implemented to perform the conceptual design shielding assessment of the proposed SNS. Biological shields have been designed and assessed for the proton beam transport system and associated beam dumps, the target station, and the target service cell and general remote maintenance cell. Shielding requirements have been assessed with respect to weight, space, and dose-rate constraints for operating, shutdown, and accident conditions. A discussion of the proposed facility design, conceptual design shielding requirements calculational strategy, source terms, preliminary results and conclusions, and recommendations for additional analyses are presented

  2. High energy halogen atom reactions activated by nuclear transformations. Progress report, February 15, 1980-February 14, 1981

    International Nuclear Information System (INIS)

    1981-02-01

    The stereochemistry of high energy 18 F, /sup 34m/Cl, and 76 Br substitution reactions involving enantiomeric molecules in the gas and condensed phase is studied. The gas to condensed state transition in halogen high energy chemistry, involving chlorine, bromine, and iodine activated by the (n,γ) and (I.T.) processes in halomethanes, saturated and unsaturated hydrocarbons is being investigated in more detail. Special attention is given to defining the nature of the enhancement yields in the condensed phase. High energy halogen reactions in liquid and frozen aqueous solutions of organic and biomolecular solutes are studied in an attempt to learn more about these reactions. The applications of high energy chemistry techniques and theory to neutron activation analysis of biological systems are being continued. Special attention is given to developing procedures for trace molecular determinations in biological systems. The applications of hot halogen atoms as indicators of solute-solute interactions in liquid and frozen aqueous solutions of halogenated bases and nucleosides are being developed. Experiments are designed to explain the mechanisms of the radioprotection offered biomolecular solutes trapped within the frozen ice lattice. Reactions of bromine and iodine activated by isomeric transition with halogenated biomolecular solutes in liquid and frozen aqueous solutions are studied. The high energy reactions of iodine with the isomers of pentene have been studied in low pressure gaseous systems employing additives and rare gas moderators and liquid systems. Reactivity of excited complex formation and structural effects of electrophilic iodine attack on the pi-bond systems are studied

  3. High energy halogen atom reactions activated by nuclear transformations. Progress report, February 15, 1980-February 14, 1981

    Energy Technology Data Exchange (ETDEWEB)

    1981-02-01

    The stereochemistry of high energy /sup 18/F, /sup 34m/Cl, and /sup 76/Br substitution reactions involving enantiomeric molecules in the gas and condensed phase is studied. The gas to condensed state transition in halogen high energy chemistry, involving chlorine, bromine, and iodine activated by the (n,..gamma..) and (I.T.) processes in halomethanes, saturated and unsaturated hydrocarbons is being investigated in more detail. Special attention is given to defining the nature of the enhancement yields in the condensed phase. High energy halogen reactions in liquid and frozen aqueous solutions of organic and biomolecular solutes are studied in an attempt to learn more about these reactions. The applications of high energy chemistry techniques and theory to neutron activation analysis of biological systems are being continued. Special attention is given to developing procedures for trace molecular determinations in biological systems. The applications of hot halogen atoms as indicators of solute-solute interactions in liquid and frozen aqueous solutions of halogenated bases and nucleosides are being developed. Experiments are designed to explain the mechanisms of the radioprotection offered biomolecular solutes trapped within the frozen ice lattice. Reactions of bromine and iodine activated by isomeric transition with halogenated biomolecular solutes in liquid and frozen aqueous solutions are studied. The high energy reactions of iodine with the isomers of pentene have been studied in low pressure gaseous systems employing additives and rare gas moderators and liquid systems. Reactivity of excited complex formation and structural effects of electrophilic iodine attack on the pi-bond systems are studied.

  4. Computational Benchmark Calculations Relevant to the Neutronic Design of the Spallation Neutron Source (SNS)

    International Nuclear Information System (INIS)

    Gallmeier, F.X.; Glasgow, D.C.; Jerde, E.A.; Johnson, J.O.; Yugo, J.J.

    1999-01-01

    The Spallation Neutron Source (SNS) will provide an intense source of low-energy neutrons for experimental use. The low-energy neutrons are produced by the interaction of a high-energy (1.0 GeV) proton beam on a mercury (Hg) target and slowed down in liquid hydrogen or light water moderators. Computer codes and computational techniques are being benchmarked against relevant experimental data to validate and verify the tools being used to predict the performance of the SNS. The LAHET Code System (LCS), which includes LAHET, HTAPE ad HMCNP (a modified version of MCNP version 3b), have been applied to the analysis of experiments that were conducted in the Alternating Gradient Synchrotron (AGS) facility at Brookhaven National Laboratory (BNL). In the AGS experiments, foils of various materials were placed around a mercury-filled stainless steel cylinder, which was bombarded with protons at 1.6 GeV. Neutrons created in the mercury target, activated the foils. Activities of the relevant isotopes were accurately measured and compared with calculated predictions. Measurements at BNL were provided in part by collaborating scientists from JAERI as part of the AGS Spallation Target Experiment (ASTE) collaboration. To date, calculations have shown good agreement with measurements

  5. Targets for neutron beam spallation sources

    International Nuclear Information System (INIS)

    Bauer, G.S.

    1980-01-01

    The meeting on Targets for Neutron Beam Spallation Sources held at the Institut fuer Festkoerperforschung at KFA Juelich on June 11 and 12, 1979 was planned as an informal get-together for scientists involved in the planning, design and future use of spallation neutron sources in Europe. These proceedings contain the papers contributed to this meeting. For further information see hints under relevant topics. (orig./FKS)

  6. Mercury purification in the megawatt liquid metal spallation target of EURISOL-DS

    CERN Document Server

    Neuhausen, Joerg; Eller, Martin; Schumann, Dorothea; Eichler, Bernd; Horn, Susanne

    High power spallation targets are going to be used extensively in future research and technical facilities such as spallation neutron sources, neutrino factories, radioactive beam facilities or accelerator driven systems for the transmutation of long-lived nuclear waste. Within EURISOL-DS, a 4 MW liquid metal spallation target is designed to provide neutrons for a fission target, where neutron rich radionuclides will be produced. For the spallation target, mercury is planned to be used as target material. A large amount of radionuclides ranging from atomic number Z=1 to 81 will be produced in the liquid metal during long term irradiation. It is planned to remove those radionuclides by chemical or physicochemical methods to reduce its radioactivity. For the development of a purification procedure, knowledge about the chemical state of the different elements present in the mixture is required. We present a general concept of applicable separation techniques in a target system and show some results of experiment...

  7. Investigation of high-energy-proton effects in aluminum

    International Nuclear Information System (INIS)

    Czajkowski, C.J.; Snead, C.L. Jr.; Todosow, M.

    1997-01-01

    Specimens of 1100 aluminum were exposed to several fluences of 23.5-GeV protons at the Brookhaven Alternating Gradient Synchrotron. Although this energy is above those currently being proposed for spallation-neutron applications, the results can be viewed as indicative of trends and other microstructural evolution with fluence that take place with high-energy proton exposures such as those associated with an increasing ratio of gas generation to dpa. TEM investigation showed significantly larger bubble size and lower density of bubbles compared with lower-energy proton results. Additional testing showed that the tensile strength increased with fluence as expected, but the microhardness decreased, a result for which an intepretation is still under investigation

  8. On-line Mass Spectrometric Study of Heavy-Ion Induced Reactions at Energies up to 86 MeV/amu

    CERN Multimedia

    2002-01-01

    The aim of the experiment was to measure isotopic distributions of Li, Na, K, Rb, Cs and Fr as reaction fragments in heavy ion collisions. In order to get an overall view of the new energy range for heavy ions available from the SC, different energies and projectile-target combinations had to be studied. The data taking status is now finished. |1|2C and |1|8O beams were used in bombarding |1|2C, |9|3Nb, |1|8|1Ta and |2|3|8U in order to look at target fragmentation, projectile fragmentation and evaporative residues of spallation processes. The experimental apparatus is composed of three parts: \\item a)~A target-oven-ionizer assembly where selective thermal diffusion and selective surface ionization takes place in order to obtain a chemical separation of the reaction products. \\item b)~The mass spectrometer where the different-mass fragments are selected. \\item c)~An electrostatic ion beam line through which the fragments are transported to a low-background area where the detector (an electron multiplier) is lo...

  9. Deep spallation of medium mass isotopes by protons

    International Nuclear Information System (INIS)

    Kolsky, K.L.; Karol, P.J.

    1993-01-01

    Spallation systematics have been extended into the deep spallation mass region. Production cross sections of scandium radioisotopes from 0.8 GeV protons on 89 Y, 92,96,100 Mo, and 130 Te targets were measured and the cross sections were used to generate isobaric yield curves at A p =47. In the latter target, this corresponds to a mass loss of >80 nucleons. At ∼10 MeV/nucleon and for products outside the multifragmentation region, this is an extreme manifestation of the spallation process. The results prove to fit smooth extrapolations from trends developed in earlier work on less deep spallation. The influence of target composition is still evident even from 130 Te, in contrast to expectations, based on evaporation considerations, that this so-called memory effect would wash out

  10. Computational methods for high-energy source shielding

    International Nuclear Information System (INIS)

    Armstrong, T.W.; Cloth, P.; Filges, D.

    1983-01-01

    The computational methods for high-energy radiation transport related to shielding of the SNQ-spallation source are outlined. The basic approach is to couple radiation-transport computer codes which use Monte Carlo methods and discrete ordinates methods. A code system is suggested that incorporates state-of-the-art radiation-transport techniques. The stepwise verification of that system is briefly summarized. The complexity of the resulting code system suggests a more straightforward code specially tailored for thick shield calculations. A short guide line to future development of such a Monte Carlo code is given

  11. Neutron PSDs for the next generation of spallation neutron sources

    CERN Document Server

    Eijk, C W

    2002-01-01

    A review of R and D for neutron PSDs to be used at anticipated new spallation neutron sources: the Time-of-Flight system facility, European Spallation Source, Spallation Neutron Source and Neutron Arena, is presented. The gas-filled detectors, scintillation detectors and hybrid systems are emphasized.

  12. Calculations of radiation damage in target, container and window materials for spallation neutron sources

    International Nuclear Information System (INIS)

    Wechsler, M.S.; Mansur, L.K.

    1996-01-01

    Radiation damage in target, container, and window materials for spallation neutron sources is am important factor in the design of target stations for accelerator-driver transmutation technologies. Calculations are described that use the LAHET and SPECTER codes to obtain displacement and helium production rates in tungsten, 316 stainless steel, and Inconel 718, which are major target, container, and window materials, respectively. Results are compared for the three materials, based on neutron spectra for NSNS and ATW spallation neutron sources, where the neutron fluxes are normalized to give the same flux of neutrons of all energies

  13. Reaction wheels for kinetic energy storage

    Science.gov (United States)

    Studer, P. A.

    1984-11-01

    In contrast to all existing reaction wheel implementations, an order of magnitude increase in speed can be obtained efficiently if power to the actuators can be recovered. This allows a combined attitude control-energy storage system to be developed with structure mounted reaction wheels. The feasibility of combining reaction wheels with energy storage wwheels is demonstrated. The power required for control torques is a function of wheel speed but this energy is not dissipated; it is stored in the wheel. The I(2)R loss resulting from a given torque is shown to be constant, independent of the design speed of the motor. What remains, in order to efficiently use high speed wheels (essential for energy storage) for control purposes, is to reduce rotational losses to acceptable levels. Progress was made in permanent magnet motor design for high speed operation. Variable field motors offer more control flexibility and efficiency over a broader speed range.

  14. Charge correlations in the breakup of gold projectiles in reactions at E/A=600 MeV

    International Nuclear Information System (INIS)

    Kreutz, P.

    1992-09-01

    In the present thesis the charge correlations in the breakup of gold projectiles in heavy ion collisions at an incident energy of E/A=600 MeV were studied. Thereby it has been proved that the sum of the charges from the projectile source under exclusion of the protons (Z bound ) is saliently suited for the classification of the nuclear reactions. At large values of Z bound we fins fission and spallation reactions. For smaller values of Z bound we observe events with an increasing number of medium-heavy fragments. Thereby the multifragment events appear in the Dalitz diagrams as a continuation of more symmetric becoming spallation events. In reactions with Z bound ≅ 35 the conditions for the formation of medium-heavy fragments are optimal and the multifragment events represent the dominating exit channel. A mean multiplicity of the medium-heavy fragments of ≅ 4 is reached. (orig./HSI) [de

  15. Study on induced radioactivity of China Spallation Neutron Source

    International Nuclear Information System (INIS)

    Wu Qingbiao; Wang Qingbin; Wu Jingmin; Ma Zhongjian

    2011-01-01

    China Spallation Neutron Source (CSNS) is the first High Energy Intense Proton Accelerator planned to be constructed in China during the State Eleventh Five-Year Plan period, whose induced radioactivity is very important for occupational disease hazard assessment and environmental impact assessment. Adopting the FLUKA code, the authors have constructed a cylinder-tunnel geometric model and a line-source sampling physical model, deduced proper formulas to calculate air activation, and analyzed various issues with regard to the activation of different tunnel parts. The results show that the environmental impact resulting from induced activation is negligible, whereas the residual radiation in the tunnels has a great influence on maintenance personnel, so strict measures should be adopted.(authors)

  16. Stress and adhesion of chromia-rich scales on ferritic stainless steels in relation with spallation

    Directory of Open Access Journals (Sweden)

    A. Galerie

    2004-03-01

    Full Text Available The relation between chromia scale spallation during oxidation or cooling down of ferritic stainless steels is generally discussed in terms of mechanical stresses induced by volume changes or differential thermal expansion. In the present paper, growth and thermal stress measurements in scales grown on different ferritic steel grades have shown that the main stress accumulation occurs during isothermal scale growth and that thermal stresses are of minor importance. However, when spallation occurs, it is always during cooling down. Steel-oxide interface undulation seems to play a major role at this stage, thus relating spallation to the metal mechanical properties, thickness and surface preparation. A major influence on spallation of the minor stabilizing elements of the steels was observed which could not be related to any difference in stress state. Therefore, an original inverted blister test was developed to derive quantitative values of the metal-oxide adhesion energy. These values clearly confirmed that this parameter was influenced by scale thickness and by minor additions, titanium greatly increasing adhesion whereas niobium decreased it.

  17. Monte Carlo simulations and experimental results on neutron production in the spallation target QUINTA irradiated with 660 MeV protons

    International Nuclear Information System (INIS)

    Khushvaktov, J.H.; Yuldashev, B.S.; Adam, J.; Vrzalova, J.; Baldin, A.A.; Furman, W.I.; Gustov, S.A.; Kish, Yu.V.; Solnyshkin, A.A.; Stegailov, V.I.; Tichy, P.; Tsoupko-Sitnikov, V.M.; Tyutyunnikov, S.I.; Zavorka, L.; Svoboda, J.; Zeman, M.; Vespalec, R.; Wagner, V.

    2017-01-01

    The activation experiment was performed using the accelerated beam of the Phasotron accelerator at the Joint Institute for Nuclear Research (JINR). The natural uranium spallation target QUINTA was irradiated with protons of energy 660 MeV. Monte Carlo simulations were performed using the FLUKA and Geant4 codes. The number of leakage neutrons from the sections of the uranium target surrounded by the lead shielding and the number of leakage neutrons from the lead shield were determined. The total number of fissions in the setup QUINTA were determined. Experimental values of reaction rates for the produced nuclei in the "1"2"7I sample were obtained, and several values of the reaction rates were compared with the results of simulations by the FLUKA and Geant4 codes. The experimentally determined fluence of neutrons in the energy range of 10-200 MeV using the (n, xn) reactions in the "1"2"7I(NaI) sample was compared with the results of simulations. Possibility of transmutation of the long-lived radionuclide "1"2"9I in the QUINTA setup was estimated. [ru

  18. Coprecipitation experiment with Sm hydroxide using a multitracer produced by nuclear spallation reaction: A tool for chemical studies with superheavy elements

    International Nuclear Information System (INIS)

    Kasamatsu, Yoshitaka; Yokokita, Takuya; Toyomura, Keigo; Shigekawa, Yudai; Haba, Hiromitsu; Kanaya, Jumpei; Huang, Minghui; Ezaki, Yutaka; Yoshimura, Takashi; Morita, Kosuke; Shinohara, Atsushi

    2016-01-01

    To establish a new methodology for superheavy element chemistry, the coprecipitation behaviors of 34 elements with samarium hydroxide were investigated using multitracer produced by a spallation of Ta. The chemical reactions were rapidly equilibrated within 10 s for many elements. In addition, these elements exhibited individual coprecipitation behaviors, and the behaviors were qualitatively related to their hydroxide precipitation behaviors. It was demonstrated that the ammine and hydroxide complex formations of superheavy elements could be investigated using the established method. - Highlights: • We established a new methodology for superheavy element (SHE) chemistry. • Coprecipitation behaviors of 34 elements with Sm hydroxide could be simultaneously investigated by using multitracer. • The complex formations were investigated from the coprecipitation behaviors. • The established method will lead to the study on various precipitates of SHEs.

  19. Spallation neutron production on thick target at saturne

    International Nuclear Information System (INIS)

    David, J.C.; David, J.C.; Varignon, C.; Borne, F.; Boudard, A.; Brochard, F.; Crespin, S.; Duchazeaubeneix, J.C.; Durand, D.; Durand, J.M.; Frehaut, J.; Hannappe, F.; Lebrun, C.; Lecolley, J.F.; Ledoux, X.; Lefebvres, F.; Legrain, R.; Leray, S.; Louvel, M.; Martinez, E.; Menard, S.; Milleret, G.; Patin, Y.; Petitbon, E.; Plouin, F.; Schapira, J.P.; Stugge, L.; Terrien, Y.; Thun, J.; Volant, C.; Whittal, D.M.

    2003-01-01

    In view of the new spallation neutron source projects, we discuss the characteristics of the neutron spectra on thick targets measured at SATURNE. Some comparisons to spallation models, and especially INCL4/ABLA implemented in the LAHET code, are done. (orig.)

  20. Integral measurements of neutron production in spallation targets

    International Nuclear Information System (INIS)

    Frehaut, J.; Deneuville, D.; Ledoux, X.; Lochard, J.P.; Longuet, J.L.; Petibon, E.; Alrick, K.; Bownan, D.; Cverna, F.; King, N.S.P.; Morgan, G.L.; Greene, G.; Hanson, A.; Snead, L.; Thompson, R.; Ward, T.

    1998-01-01

    Measurements of neutron production for thick iron, tungsten and lead targets of different diameter prototypic for spallation systems have been made at SATURNE in an incident proton energy range from 400 MeV to 2 GeV. TIERCE code system calculations are in good agreement with experiment for iron and large diameter tungsten and lead targets. They overestimate the measured neutron production for tungsten and lead targets for diameter ≤20 cm. (author)

  1. Plutonium characterisation with prompt high energy gamma-rays from (n,gamma) reactions for nuclear warhead dismantlement verification

    Energy Technology Data Exchange (ETDEWEB)

    Postelt, Frederik; Gerald, Kirchner [Carl Friedrich von Weizsaecker-Centre for Science and Peace Research, Hamburg (Germany)

    2015-07-01

    Measurements of neutron induced gammas allow the characterisation of fissile material (i.e. plutonium and uranium), despite self- and additional shielding. Most prompt gamma-rays from radiative neutron capture reactions in fissile material have energies between 3 and 6.5 MeV. Such high energy photons have a high penetrability and therefore minimise shielding and self-absorption effects. They are also isotope specific and therefore well suited to determine the isotopic composition of fissile material. As they are non-destructive, their application in dismantlement verification is desirable. Disadvantages are low detector efficiencies at high gamma energies, as well as a high background of gammas which result from induced fission reactions in the fissile material, as well as delayed gammas from both, (n,f) and(n,gamma) reactions. In this talk, simulations of (n,gamma) measurements and their implications are presented. Their potential for characterising fissile material is assessed and open questions are addressed.

  2. Lattice design of medium energy beam transport line for n spallation neutron source

    International Nuclear Information System (INIS)

    Dhingra, Rinky; Kulkarni, Nita S.; Kumar, Vinit

    2015-01-01

    A 1 GeV H - injector linac is being designed at RRCAT for the proposed Indian Spallation Neutron Source (ISNS). The front-end of the injector linac will consist of Radiofrequency Quadrupole (RFQ) linac, which will accelerate the H - beam from 50 keV to 3 MeV. The beam will be further accelerated in superconducting Single Spoke Resonators (SSRs). A Medium Energy Beam Transport (MEBT) line will be used to transport the beam from the exit of RFQ to the input of SSR. The main purpose of MEBT is to carry out beam matching from RFQ to SSR, and beam chopping. In this paper, we describe the optimization criteria for the lattice design of MEBT. The optimized lattice element parameters are presented for zero and full (15 mA) current case. Beam dynamics studies have been carried out using an envelope tracing code Trace-3D. Required beam deflection angle due to the chopper housed inside the MEBT for beam chopping has also been estimated. (author)

  3. Analysis of the proton-induced reactions at 150 MeV - 24 GeV by high energy nuclear reaction code JAM

    International Nuclear Information System (INIS)

    Niita, Koji; Nara, Yasushi; Takada, Hiroshi; Nakashima, Hiroshi; Chiba, Satoshi; Ikeda, Yujiro

    1999-09-01

    We are developing a nucleon-meson transport code NMTC/JAM, which is an upgraded version of NMTC/JAERI. NMTC/JAM implements the high energy nuclear reaction code JAM for the infra-nuclear cascade part. By using JAM, the upper limits of the incident energies in NMTC/JAERI, 3.5 GeV for nucleons and 2.5 GeV for mesons, are increased drastically up to several hundreds GeV. We have modified the original JAM code in order to estimate the residual nucleus and its excitation energy for nucleon or pion induced reactions by assuming a simple model for target nucleus. As a result, we have succeeded in lowering the applicable energies of JAM down to about 150 MeV. In this report, we describe the main components of JAM code, which should be implemented in NMTC/JAM, and compare the results calculated by JAM code with the experimental data and with those by LAHET2.7 code for proton induced reactions from 150 MeV to several 10 GeV. It has been found that the results of JAM can reproduce quite well the experimental double differential cross sections of neutrons and pions emitted from the proton induced reactions from 150 MeV to several 10 GeV. On the other hand, the results of LAHET2.7 show the strange behavior of the angular distribution of nucleons and pions from the reactions above 4 GeV. (author)

  4. Spallation Neutron Source High Power RF Installation and Commissioning Progress

    CERN Document Server

    McCarthy, Michael P; Bradley, Joseph T; Fuja, Ray E; Gurd, Pamela; Hardek, Thomas; Kang, Yoon W; Rees, Daniel; Roybal, William; Young, Karen A

    2005-01-01

    The Spallation Neutron Source (SNS) linac will provide a 1 GeV proton beam for injection into the accumulator ring. In the normal conducting (NC) section of this linac, the Radio Frequency Quadupole (RFQ) and six drift tube linac (DTL) tanks are powered by seven 2.5 MW, 402.5 MHz klystrons and the four coupled cavity linac (CCL) cavities are powered by four 5.0 MW, 805 MHz klystrons. Eighty-one 550 kW, 805 MHz klystrons each drive a single cavity in the superconducting (SC) section of the linac. The high power radio frequency (HPRF) equipment was specified and procured by LANL and tested before delivery to ensure a smooth transition from installation to commissioning. Installation of RF equipment to support klystron operation in the 350-meter long klystron gallery started in June 2002. The final klystron was set in place in September 2004. Presently, all RF stations have been installed and high power testing has been completed. This paper reviews the progression of the installation and testing of the HPRF Sys...

  5. Spallation Neutron Source (SNS)

    Data.gov (United States)

    Federal Laboratory Consortium — The SNS at Oak Ridge National Laboratory is a next-generation spallation neutron source for neutron scattering that is currently the most powerful neutron source in...

  6. Study on bulk shielding for a spallation neutron source facility in the high-intensity proton accelerator project

    CERN Document Server

    Maekawa, F; Takada, H; Teshigawara, M; Watanabe, N

    2002-01-01

    Under the JAERI-KEK High-Intensity Proton Accelerator Project, a spallation neutron source driven by a 3 GeV-1 MW proton beam is planed to be constructed in a main part of the Materials and Life Science Facility. This report describes results of a study on bulk shielding performance of a biological shield for the spallation neutron source by means of a Monte Carlo calculation method, that is important in terms of radiation safety and cost reduction. A shielding configuration was determined as a reference case by considering preliminary studies and interaction with other components, then shielding thickness that was required to achieve a target dose rate of 1 mu Sv/h was derived. Effects of calculation conditions such as shielding materials and dimensions on the shielding performance was investigated by changing those parameters. By taking all the results and design margins into account, a shielding configuration that was identified as the most appropriate was finally determined as follows. An iron shield regi...

  7. Probing nuclei with high-energy hadronic reactions

    International Nuclear Information System (INIS)

    Moss, J.M.

    1995-01-01

    I review the subject of hadron-nucleus collisions at energies where peturbative theory is applicable. Reactions studied experimentally at the Fermilab Tevatron and CERN's Super Proton Synchrotron include the Drell-Yan Process, direct photon production, quarkonium production, and open charm production. I conclude with an observation about a new era of proton-nucleus and nucleus-nucleus experiments which will be carried out at the hadron colliders, RHIC and LHC

  8. A comparison of microstructures in copper irradiated with fission, fusion, and spallation neutrons

    International Nuclear Information System (INIS)

    Muroga, T.; Heinisch, H.L.; Sommer, W.F.; Ferguson, P.D.

    1992-01-01

    The objective of this work is to investigate the effects of the neutron energy spectrum in low dose irradiations on the microstructure and mechanical properties of metals. The microstructures of pure copper irradiated to low doses at 36-90 C with spallation neutrons, fusion neutrons and fission neutrons are compared. The defect cluster densities for the spallation and fusion neutrons are very similar when compared on the basis of displacements per atom (dpa). In both cases, the density increases in proportion to the square root of the dpa. The difference in defect density between fusion neutrons and fission neutrons corresponds with differences observed in data on yield stress changes

  9. Preliminary radiation transport analysis for the proposed National Spallation Neutron Source (NSNS)

    International Nuclear Information System (INIS)

    Johnson, J.O.; Lillie, R.A.

    1997-01-01

    The use of neutrons in science and industry has increased continuously during the past 50 years with applications now widely used in physics, chemistry, biology, engineering, and medicine. Within this history, the relative merits of using pulsed accelerator spallation sources versus reactors for neutron sources as the preferred option for the future. To address this future need, the Department of Energy (DOE) has initiated a pre-conceptual design study for the National Spallation Neutron Source (NSNS) and given preliminary approval for the proposed facility to be built at Oak Ridge National Laboratory (ORNL). The DOE directive is to design and build a short pulse spallation source in the 1 MS power range with sufficient design flexibility that it can be upgraded and operated at a significantly higher power at a later stage. The pre-conceptualized design of the NSNS initially consists of an accelerator system capable of delivering a 1 to 2 GeV proton beam with 1 MW of beam power in an approximate 0.5 microsecond pulse at a 60 Hz frequency onto a single target station. The NSNS will be upgraded in stages to a 5 MW facility with two target stations (a high power station operating at 60 Hz and a low power station operating at 10 Hz). Each target station will contain four moderators (combinations of cryogenic and ambient temperature) and 18 beam liens for a total of 36 experiment stations. This paper summarizes the radiation transport analysis strategies for the proposed NSNS facility

  10. The BLAIRR Irradiation Facility Hybrid Spallation Target Optimization

    Energy Technology Data Exchange (ETDEWEB)

    Simos N.; Hanson A.; Brown, D.; Elbakhshawn, M.

    2016-04-11

    BLAIRR STUDY STATUS OVERVIEW Beamline Complex Evaluation/Assessment and Adaptation to the Goals Facility Radiological Constraints ? Large scale analyses of conventional facility and integrated shield (concrete, soil)Target Optimization and Design: Beam-target interaction optimization Hadronic interaction and energy deposition limitations Single phase and Hybrid target concepts Irradiation Damage Thermo-mechanical considerations Spallation neutron fluence optimization for (a) fast neutron irradiation damage (b) moderator/reflector studies, (c) NTOF potential and optimization (d) mono-energetic neutron beam

  11. Experimental studies of spallation on thin target

    International Nuclear Information System (INIS)

    Borne, F.; Crespin, S.; Drake, D.; Frehaut, J.; Ledoux, X.; Lochard, J.P.; Martinez, E.; Patin, Y.; Petibon, E.; Pras, Ph.; Boudard, A.; Legrain, R.; Leray, S.; Terrien, Y.; Bouyer, P.; Brochard, F.; Duchazeaubeneix, J.C.; Durand, J.M.; Meigo, S.I.; Milleret, G.; Thun, J.; Whittal, D.M.; Wlazlo, W.; Lebrun, C.; Lecolley, J.F.; Lecolley, F.R.; Lefebvres, F.; Louvel, M.; Varignon, C.; Menard, S.; Stugge, L.; Hanappe, F.

    2000-01-01

    Angular distribution of spallation neutrons induced by protons (0.8, 1.2 and 1.6 GeV) and deuterons (0.8 and 1.6 GeV beams on various thin targets have been measured at SATURNE (CEA Saclay/France) with two complementary experimental techniques: the time-of-flight measurement with tagged incident protons for low energy neutrons (2-400 MeV) and the use of a hydrogen converter associated are analysed, interpreted and finally compared with theoretical previsions of simulation codes using the TIERCE system including the intranuclear cascade codes of BERTINI and CUGNON. (authors)

  12. Irradiation damage of ferritic/martensitic steels: Fusion program data applied to a spallation neutron source

    International Nuclear Information System (INIS)

    Klueh, R.L.

    1997-01-01

    Ferritic/martensitic steels were chosen as candidates for future fusion power plants because of their superior swelling resistance and better thermal properties than austenitic stainless steels. For the same reasons, these steels are being considered for the target structure of a spallation neutron source, where the structural materials will experience even more extreme irradiation conditions than expected in a fusion power plant first wall (i.e., high-energy neutrons that produce large amounts of displacement damage and transmutation helium). Extensive studies on the effects of neutron irradiation on the mechanical properties of ferritic/martensitic steels indicate that the major problem involves the effect of irradiation on fracture, as determined by a Charpy impact test. There are indications that helium can affect the impact behavior. Even more helium will be produced in a spallation neutron target material than in the first wall of a fusion power plant, making helium effects a prime concern for both applications. 39 refs., 10 figs

  13. Radiation protection of the operation of accelerator facilities. On high energy proton and electron accelerators

    International Nuclear Information System (INIS)

    Kondo, Kenjiro

    1997-01-01

    Problems in the radiation protection raised by accelerated particles with energy higher than several hundreds MeV in strong accelerator facilities were discussed in comparison with those with lower energy in middle- and small-scale facilities. The characteristics in the protection in such strong accelerator facilities are derived from the qualitative changes in the interaction between the high energy particles and materials and from quantitative one due to the beam strength. In the former which is dependent on the emitting mechanism of the radiation, neutron with broad energy spectrum and muon are important in the protection, and in the latter, levels of radiation and radioactivity which are proportional to the beam strength are important. The author described details of the interaction between high energy particles and materials: leading to the conclusion that in the electron accelerator facilities, shielding against high energy-blemsstrahlung radiation and -neutron is important and in the proton acceleration, shielding against neutron is important. The characteristics of the radiation field in the strong accelerator facilities: among neutron, ionized particles and electromagnetic wave, neutron is most important in shielding since it has small cross sections relative to other two. Considerations for neutron are necessary in the management of exposure. Multiplicity of radionuclides produced: which is a result of nuclear spallation reaction due to high energy particles, especially to proton. Radioactivation of the accelerator equipment is a serious problem. Other problems: the interlock systems, radiation protection for experimenters and maintenance of the equipment by remote systems. (K.H.). 11 refs

  14. (3He,α) reaction mechanism at high energy and neutron inner shell structure

    International Nuclear Information System (INIS)

    Wiele, J. van de.

    1980-01-01

    The ( 3 He,α) reaction on 12 C, 16 O, 28 Si, 58 Ni, 90 Zr, 118 Sn, 124 Sn and 208 Pb targets has been studied at Esub( 3 He) = 217 MeV (or 205 MeV) in order to investigate the reaction mechanism at high energy and large momentum transfer. The reaction yields large cross sections at very forward angles and strongly enhances the largest orbital momentum transfer. The angular distribution shapes are well reproduced in the frame-work of the Z-R- D.W.B.A. analysis if we use a unique empirical α-potential: Vsub(α)(Esub(α)) = Vsub( 3 He)(3/4 Esub(α)) + Vsub(n)(1/4 Esub(α)). The excitation energy spectra have been measured up to 100 MeV in the residual light and medium nuclei and up to about 16 MeV in heavy nuclei. In addition to the well-known low-lying levels, peaks or broad structures are observed for each nucleus at higher excitation energies. They are attributed to pick up from inner shells: 1s( 11 C and 15 O), 1p( 27 Si), 1d5/2 + 1p( 57 Ni), 1f7/2( 89 Zr) 1g9/2 117 Sn, 123 Sn and 1h11/2( 207 Pb). Selectivity and localization of direct and indirect pick up ( 3 He,α) reactions were studied. Finite range calculations show that this reaction is not very sensitive to the details of the range from function but only to D 0 coefficient and range R. A microscopic α-nucleus optical potential calculated with n-n dependent and independent density forces is able to reproduce both elastic scattering and pick up reaction angular distributions [fr

  15. Spallation symbiont and thorium breeding

    International Nuclear Information System (INIS)

    Furukawa, Kazuo

    1991-01-01

    The medium term world energy and environment countermeasures for 2020-2070 are not yet clearly established. The forecast of energy situation hereafter, its problems and the measures for solution are considered. World trend is removing borders, and the north-south problems are increasing the importance. The rational and clear idea with the support of concrete technology is required. The demand of energy will increase enormously at the annual rate of 2.3%. The world energy situation was forecast considering the increase of population, and it will be 115 TW at the end of the next century. The present status, problems and the countermeasures in nuclear fission energy technology are explained. The countermeasures should be based on three principles, namely Th-U-233 cycle, the utilization of molten fluoride fuel medium and the separation of molten salt breeders and molten salt reactors. Accelerator molten salt breeders, small molten salt reactors, the nuclear fuel cycle and the annihilation process for radioactive wastes are reported. The perspective that the nuclear energy system, in which the reactor safety, the measures to wastes and others are improved by the spallation-fission symbiont using thorium molten salt as the working medium, can be constructed is shown. (K.I.)

  16. Linac design for the European spallation source

    Energy Technology Data Exchange (ETDEWEB)

    Klein, H. [Universitaet Postfach, Frankfurt am Main (Germany)

    1995-10-01

    A study group has started to develop a conceptual design for a European Spallation Source (ESS). This pulsed 5 MW source presently consists of a 1.334 GeV linac and two compressor rings. In the following mainly the high intensity linac part will be discussed, which has some features of interest for accelerators for transmutation of radioactive waste too.

  17. Study of the Energy Dependence of the Anomalous Mean Free Path Effect by Means of High-energy ($\\geq$12 GeV/nucleon) Helium Nuclei

    CERN Multimedia

    2002-01-01

    The proposal concerns an extension to higher energies of previous experiments which have provided evidence for anomalously short reaction mean free paths among projectile fragments from heavy ion interactions.\\\\ \\\\ It is intended to provide information on the interaction properties of projectile fragments, mainly 3He, P, D, T as well as of scattered 4He nuclei in passive detectors exposed to beams of energies exceeding those available in previous experim factor of about 7. \\\\ \\\\ Interaction mean free paths and event topologies will be measured in a nuclear emulsion stack (LBL) of 7.5~cm~x~5~cm~x~25~cm dimensions. Decay effects will be recorded by comparing the activity of spallation residues in dense and diluted copper target assemblies (Marburg). Target fragmentation will be studied in a stack of silverchloride crystal foils (Frankfurt) of about 7~cm~x~6~cm~x~1~cm dimensions. The \\alpha beam ejected at EJ~62 will be used to provide both exposures at high intensity of 10|1|2 alphas on th and at low intensity ...

  18. A medium energy neutron deep penetration experiment

    International Nuclear Information System (INIS)

    Amian, W.; Cloth, P.; Druecke, V.; Filges, D.; Paul, N.; Schaal, H.

    1986-11-01

    A deep penetration experiment conducted at the Los Alamos WNR facility's Spallation Neutron Target is compared with calculations using intra-nuclear-cascade and S N -transport codes installed at KFA-IRE. In the experiment medium energy reactions induced by neutrons between 15 MeV and about 150 MeV inside a quasi infinite slab of iron have been measured using copper foil monitors. Details of the experimental procedure and the theoretical methods are described. A comparison of absolute reaction rates for both experimentally and theoretically derived reactions is given. The present knowledge of the corresponding monitor reaction cross sections is discussed. (orig.)

  19. Neutron diffractometers for structural biology at spallation neutron sources

    International Nuclear Information System (INIS)

    Schoenborn, B.P.; Pitcher, E.

    1994-01-01

    Spallation neutron sources are ideal for diffraction studies of proteins and oriented molecular complexes. With spoliation neutrons and their time dependent wavelength structure, it is easy to electronically select data with an optimal wavelength bandwidth and cover the whole Laue spectrum as time (wavelength) resolved snapshots. This optimized data quality with best peak-to-background ratios and provides adequate spatial and energy resolution to eliminate peak overlaps. The application of this concept will use choppers to select the desired Laue wavelength spectrum and employ focusing optics and large cylindrical 3 He detectors to optimize data collection rates. Such a diffractometer will cover a Laue wavelength range from 1 to 5 Angstrom with a flight path length of 10m and an energy resolution of 0.25 Angstrom. Moderator concepts for maximal flux distribution within this energy range will be discussed using calculated flux profiles. Since the energy resolution required for such timed data collection in this super Laue techniques is not very high, the use of a linac only (LAMPF) spoliation target is an exciting possibility with an order of magnitude increase in flux

  20. Neutron diffractometers for structural biology at spallation neutron sources

    Energy Technology Data Exchange (ETDEWEB)

    Schoenborn, B.P.; Pitcher, E. [Los Alamos National Laboratory, NM (United States)

    1994-12-31

    Spallation neutron sources are ideal for diffraction studies of proteins and oriented molecular complexes. With spoliation neutrons and their time dependent wavelength structure, it is easy to electronically select data with an optimal wavelength bandwidth and cover the whole Laue spectrum as time (wavelength) resolved snapshots. This optimized data quality with best peak-to-background ratios and provides adequate spatial and energy resolution to eliminate peak overlaps. The application of this concept will use choppers to select the desired Laue wavelength spectrum and employ focusing optics and large cylindrical {sup 3}He detectors to optimize data collection rates. Such a diffractometer will cover a Laue wavelength range from 1 to 5{Angstrom} with a flight path length of 10m and an energy resolution of 0.25{Angstrom}. Moderator concepts for maximal flux distribution within this energy range will be discussed using calculated flux profiles. Since the energy resolution required for such timed data collection in this super Laue techniques is not very high, the use of a linac only (LAMPF) spoliation target is an exciting possibility with an order of magnitude increase in flux.

  1. Complementarity of long pulse and short pulse spallation sources

    Energy Technology Data Exchange (ETDEWEB)

    Mezei, F [Hahn-Meitner-Institut Berlin GmbH (Germany)

    1995-11-01

    The complementarity of short pulse spallation sources (SPSS) and steady state (CW) reactors is a widely accepted concept. SPSS and long pulse spallation sources (LPSS) are complementary in two ways: (a) in their performance in neutron scattering experiments LPSS closely emulate CW reactors. In this respect two facets of the time-of-flight (TOF) monochromator method adequate for LPSS will be discussed: the superiority of the TOF approach to the crystal monochromator method in high resolution powder diffraction, and the novel technique of repetition rate multiplication in TOF spectroscopy, (b) LPSS combined with adequate chopper systems can also emulate SPSS in a number of applications. It will be shown that the LPSS method of producing short neutron pulses is more efficient for cold and thermal neutrons (below an energy of about 100 MeV), while SPSS is the more favourable approach for hot, epithermal neutrons, i.e. in the slowing down regime in contrast to the moderated regime. These two aspects of complementarity of LPSS and SPSS lead to the conclusions that for about 75% of the spectrum of neutron scattering experiments as known of today the LPSS approach is the most advantageous one with a feasible neutron intensity exceeding that available at ILL by a factor of about 30, while for the remaining 25% of applications the SPSS technique is superior with a well-known potential of a similar gain over present day performances. (author) 7 figs., 6 refs.

  2. Complementarity of long pulse and short pulse spallation sources

    International Nuclear Information System (INIS)

    Mezei, F.

    1995-01-01

    The complementarity of short pulse spallation sources (SPSS) and steady state (CW) reactors is a widely accepted concept. SPSS and long pulse spallation sources (LPSS) are complementary in two ways: a) in their performance in neutron scattering experiments LPSS closely emulate CW reactors. In this respect two facets of the time-of-flight (TOF) monochromator method adequate for LPSS will be discussed: the superiority of the TOF approach to the crystal monochromator method in high resolution powder diffraction, and the novel technique of repetition rate multiplication in TOF spectroscopy, b) LPSS combined with adequate chopper systems can also emulate SPSS in a number of applications. It will be shown that the LPSS method of producing short neutron pulses is more efficient for cold and thermal neutrons (below an energy of about 100 MeV), while SPSS is the more favourable approach for hot, epithermal neutrons, i.e. in the slowing down regime in contrast to the moderated regime. These two aspects of complementarity of LPSS and SPSS lead to the conclusions that for about 75% of the spectrum of neutron scattering experiments as known of today the LPSS approach is the most advantageous one with a feasible neutron intensity exceeding that available at ILL by a factor of about 30, while for the remaining 25% of applications the SPSS technique is superior with a well-known potential of a similar gain over present day performances. (author) 7 figs., 6 refs

  3. High energy halogen atom reactions activated by nuclear transformations. Progress report, February 15, 1979-February 14, 1980

    Energy Technology Data Exchange (ETDEWEB)

    Rack, E.P.

    1980-02-01

    The program consists of six interrelated areas: (1) Reactions of iodine with alkenes and alkynes activated by radiative neutron capture and isomeric transition in low pressure gaseous systems employing additives and rare gas moderators, high pressure, and liquid systems. Special attention was given to the reactivity of excited complex formation and structural effects of electrophilic iodine attack on various pi-bond systems. (2) The gas-to-condensed phase transition in halogen high energy chemistry. Current interest involves the study of caging effects of an ice lattice on recombination reactions involving neutron-irradiated frozen aqueous solutions of halogenated organic and biochemical solutes in order to learn more about kinetic energy effects, halogen size, solute molecule size, steric effects and hydrogen bonding within an ice lattice cage. (3) Systematics of halogen hot atom reactions. The reactions of /sup 80m/Br, /sup 80/Br, /sup 82m/Br + /sup 82/Br, /sup 82/Br, /sup 82/Br, /sup 128/I, /sup 130/I, and /sup 130m/I + /sup 130/I activated by radiative neutron capture or isomeric transition in hydrocarbons and halo-substituted alkanes in low pressure and high pressure gaseous systems employing additives and rare gas moderators are currently being studied. (4) Mathematical and computer simulation studies of caging events within an ice lattice are being investigated. (5) At Brookhaven National Laboratory, cyclotron-produced chlorine and fluorine hot atoms substitution reactions with molecules possessing a single chiral center are under investigation to determine the role of hot atom kinetic energy, halogen atom, enantioner structure, steric effects and phase on the extent of substitution by retention of configuration or by Walden inversion. (6) The applications of high energy techniques and concepts to neutron activation analysis for trace element determinations in biological systems was continued.

  4. The search for high-energy deuterons in the 3He +3He reaction

    International Nuclear Information System (INIS)

    Pigeon, R.; Slobodrian, R.J.

    1979-01-01

    High-energy deuterons have been detected from the 3 He + 3 He reaction with a system sensitive to cross-sections of 0.6 nb sr -1 . Several tests have permitted to evaluate the small contribution of spurious events. The deuterons are kenematically consistent with the reaction 3 He + 3 He→ 2 H + 4 He + e + +ν, but the measured cross-section at 20deg laboratory is too high for a weak-interaction process; (1.3 +- 0.2) nb sr -1 . It might be due to an interaction of intermediate strength causing the decay of pp pairs ( 3 He) into deuterons. Other alternatives and the implications concerning fusion processes and the production of neutrinos in the sun are discussed in the text

  5. High energy halogen atom reactions activated by nuclear transformations. Progress report, February 15, 1979-February 14, 1980

    International Nuclear Information System (INIS)

    Rack, E.P.

    1980-02-01

    The program consists of six interrelated areas: (1) Reactions of iodine with alkenes and alkynes activated by radiative neutron capture and isomeric transition in low pressure gaseous systems employing additives and rare gas moderators, high pressure, and liquid systems. Special attention was given to the reactivity of excited complex formation and structural effects of electrophilic iodine attack on various pi-bond systems. (2) The gas-to-condensed phase transition in halogen high energy chemistry. Current interest involves the study of caging effects of an ice lattice on recombination reactions involving neutron-irradiated frozen aqueous solutions of halogenated organic and biochemical solutes in order to learn more about kinetic energy effects, halogen size, solute molecule size, steric effects and hydrogen bonding within an ice lattice cage. (3) Systematics of halogen hot atom reactions. The reactions of /sup 80m/Br, 80 Br, /sup 82m/Br + 82 Br, 82 Br, 82 Br, 128 I, 130 I, and /sup 130m/I + 130 I activated by radiative neutron capture or isomeric transition in hydrocarbons and halo-substituted alkanes in low pressure and high pressure gaseous systems employing additives and rare gas moderators are currently being studied. (4) Mathematical and computer simulation studies of caging events within an ice lattice are being investigated. (5) At Brookhaven National Laboratory, cyclotron-produced chlorine and fluorine hot atoms substitution reactions with molecules possessing a single chiral center are under investigation. (6) The applications of high energy techniques and concepts to neutron activation analysis for trace elements and trace molecule determinations in biological systems was continued

  6. Qualification tests of materials for spallation neutron sources

    International Nuclear Information System (INIS)

    Sommer, W.F.; Maloy, S.; Wechsler, M.S.

    1997-01-01

    Several laboratories will take part in an extensive materials qualification program that includes irradiation in the proton beam and neutron field available at the Los Alamos Spallation Radiation Damage Facility (LASREF). A number of candidate materials will be exposed to prototypic spallation producing particle radiation. Studies of corrosion-related phenomena and the mitigation of these effects will also be accomplished

  7. The Spallation Neutron Source accelerator system design

    Science.gov (United States)

    Henderson, S.; Abraham, W.; Aleksandrov, A.; Allen, C.; Alonso, J.; Anderson, D.; Arenius, D.; Arthur, T.; Assadi, S.; Ayers, J.; Bach, P.; Badea, V.; Battle, R.; Beebe-Wang, J.; Bergmann, B.; Bernardin, J.; Bhatia, T.; Billen, J.; Birke, T.; Bjorklund, E.; Blaskiewicz, M.; Blind, B.; Blokland, W.; Bookwalter, V.; Borovina, D.; Bowling, S.; Bradley, J.; Brantley, C.; Brennan, J.; Brodowski, J.; Brown, S.; Brown, R.; Bruce, D.; Bultman, N.; Cameron, P.; Campisi, I.; Casagrande, F.; Catalan-Lasheras, N.; Champion, M.; Champion, M.; Chen, Z.; Cheng, D.; Cho, Y.; Christensen, K.; Chu, C.; Cleaves, J.; Connolly, R.; Cote, T.; Cousineau, S.; Crandall, K.; Creel, J.; Crofford, M.; Cull, P.; Cutler, R.; Dabney, R.; Dalesio, L.; Daly, E.; Damm, R.; Danilov, V.; Davino, D.; Davis, K.; Dawson, C.; Day, L.; Deibele, C.; Delayen, J.; DeLong, J.; Demello, A.; DeVan, W.; Digennaro, R.; Dixon, K.; Dodson, G.; Doleans, M.; Doolittle, L.; Doss, J.; Drury, M.; Elliot, T.; Ellis, S.; Error, J.; Fazekas, J.; Fedotov, A.; Feng, P.; Fischer, J.; Fox, W.; Fuja, R.; Funk, W.; Galambos, J.; Ganni, V.; Garnett, R.; Geng, X.; Gentzlinger, R.; Giannella, M.; Gibson, P.; Gillis, R.; Gioia, J.; Gordon, J.; Gough, R.; Greer, J.; Gregory, W.; Gribble, R.; Grice, W.; Gurd, D.; Gurd, P.; Guthrie, A.; Hahn, H.; Hardek, T.; Hardekopf, R.; Harrison, J.; Hatfield, D.; He, P.; Hechler, M.; Heistermann, F.; Helus, S.; Hiatt, T.; Hicks, S.; Hill, J.; Hill, J.; Hoff, L.; Hoff, M.; Hogan, J.; Holding, M.; Holik, P.; Holmes, J.; Holtkamp, N.; Hovater, C.; Howell, M.; Hseuh, H.; Huhn, A.; Hunter, T.; Ilg, T.; Jackson, J.; Jain, A.; Jason, A.; Jeon, D.; Johnson, G.; Jones, A.; Joseph, S.; Justice, A.; Kang, Y.; Kasemir, K.; Keller, R.; Kersevan, R.; Kerstiens, D.; Kesselman, M.; Kim, S.; Kneisel, P.; Kravchuk, L.; Kuneli, T.; Kurennoy, S.; Kustom, R.; Kwon, S.; Ladd, P.; Lambiase, R.; Lee, Y. Y.; Leitner, M.; Leung, K.-N.; Lewis, S.; Liaw, C.; Lionberger, C.; Lo, C. C.; Long, C.; Ludewig, H.; Ludvig, J.; Luft, P.; Lynch, M.; Ma, H.; MacGill, R.; Macha, K.; Madre, B.; Mahler, G.; Mahoney, K.; Maines, J.; Mammosser, J.; Mann, T.; Marneris, I.; Marroquin, P.; Martineau, R.; Matsumoto, K.; McCarthy, M.; McChesney, C.; McGahern, W.; McGehee, P.; Meng, W.; Merz, B.; Meyer, R.; Meyer, R.; Miller, B.; Mitchell, R.; Mize, J.; Monroy, M.; Munro, J.; Murdoch, G.; Musson, J.; Nath, S.; Nelson, R.; Nelson, R.; O`Hara, J.; Olsen, D.; Oren, W.; Oshatz, D.; Owens, T.; Pai, C.; Papaphilippou, I.; Patterson, N.; Patterson, J.; Pearson, C.; Pelaia, T.; Pieck, M.; Piller, C.; Plawski, T.; Plum, M.; Pogge, J.; Power, J.; Powers, T.; Preble, J.; Prokop, M.; Pruyn, J.; Purcell, D.; Rank, J.; Raparia, D.; Ratti, A.; Reass, W.; Reece, K.; Rees, D.; Regan, A.; Regis, M.; Reijonen, J.; Rej, D.; Richards, D.; Richied, D.; Rode, C.; Rodriguez, W.; Rodriguez, M.; Rohlev, A.; Rose, C.; Roseberry, T.; Rowton, L.; Roybal, W.; Rust, K.; Salazer, G.; Sandberg, J.; Saunders, J.; Schenkel, T.; Schneider, W.; Schrage, D.; Schubert, J.; Severino, F.; Shafer, R.; Shea, T.; Shishlo, A.; Shoaee, H.; Sibley, C.; Sims, J.; Smee, S.; Smith, J.; Smith, K.; Spitz, R.; Staples, J.; Stein, P.; Stettler, M.; Stirbet, M.; Stockli, M.; Stone, W.; Stout, D.; Stovall, J.; Strelo, W.; Strong, H.; Sundelin, R.; Syversrud, D.; Szajbler, M.; Takeda, H.; Tallerico, P.; Tang, J.; Tanke, E.; Tepikian, S.; Thomae, R.; Thompson, D.; Thomson, D.; Thuot, M.; Treml, C.; Tsoupas, N.; Tuozzolo, J.; Tuzel, W.; Vassioutchenko, A.; Virostek, S.; Wallig, J.; Wanderer, P.; Wang, Y.; Wang, J. G.; Wangler, T.; Warren, D.; Wei, J.; Weiss, D.; Welton, R.; Weng, J.; Weng, W.-T.; Wezensky, M.; White, M.; Whitlatch, T.; Williams, D.; Williams, E.; Wilson, K.; Wiseman, M.; Wood, R.; Wright, P.; Wu, A.; Ybarrolaza, N.; Young, K.; Young, L.; Yourd, R.; Zachoszcz, A.; Zaltsman, A.; Zhang, S.; Zhang, W.; Zhang, Y.; Zhukov, A.

    2014-11-01

    The Spallation Neutron Source (SNS) was designed and constructed by a collaboration of six U.S. Department of Energy national laboratories. The SNS accelerator system consists of a 1 GeV linear accelerator and an accumulator ring providing 1.4 MW of proton beam power in microsecond-long beam pulses to a liquid mercury target for neutron production. The accelerator complex consists of a front-end negative hydrogen-ion injector system, an 87 MeV drift tube linear accelerator, a 186 MeV side-coupled linear accelerator, a 1 GeV superconducting linear accelerator, a 248-m circumference accumulator ring and associated beam transport lines. The accelerator complex is supported by ~100 high-power RF power systems, a 2 K cryogenic plant, ~400 DC and pulsed power supply systems, ~400 beam diagnostic devices and a distributed control system handling ~100,000 I/O signals. The beam dynamics design of the SNS accelerator is presented, as is the engineering design of the major accelerator subsystems.

  8. The WNR facility - a pulsed spallation neutron source at the Los Alamos Scientific Laboratory

    International Nuclear Information System (INIS)

    Russell, G.J.; Lisowski, P.W.; King, N.S.P.

    1978-01-01

    The Weapons Neutron Research facility (WNR) at the Los Alamos Scientific Laboratory is the first operating example of a new class of pulsed neutron sources using the X(p,n)Y spallation reaction. At present, up to 10 microamperes of 800-MeV protons from the Clinton P. Anderson Meson Physics Facility (LAMPF) linear accelerator bombard a Ta target to produce an intense white-neutron spectrum from about 800 MeV to 100 keV. The Ta target can be coupled with CH 2 and H 2 O moderators to produce neutrons of lower energy. The time structure of the WNR proton beam may be varied to optimize neutron time-of-flight (TOF) measurements covering the energy range from several hundred MeV to a few meV. The neutronics of the WNR target and target/moderator configurations have been calculated from 800 MeV to 0.5 eV. About 11 neutrons per proton are predicted for the existing Ta target. Some initial neutron TOF data are presented and compared with calculations

  9. MEGAPIE-TEST: A European Project on Spallation Target Testing

    International Nuclear Information System (INIS)

    Knebel, Joachim U.; Klein, Jean-Christophe; Gorse, Dominique; Agostini, Pietro; Groeschel, Friedrich; Kupschus, Peter; Kirchner, Thomas; Vogt, Jean-Bernard

    2002-01-01

    Within the Euratom 5. Framework Programme (5FP) the European Commission is funding the MEGAPIE-TEST Project (Megawatt Pilot Experiment - Testing) over a period of three years, starting in September 2001. The project is combining the efforts of 8 main associations. MEGAPIE is a liquid metal spallation target of 1 MW of beam power. The main results of the MEGAPIE-TEST project will be: Development and comprehensive testing of a liquid metal spallation target both under beam-off and beam-on conditions, and the set up of a handbook on the design of a neutron spallation source in general. The operation of MEGAPIE within the accelerator complex SINQ at Paul Scherrer Institute (PSI), Switzerland, is envisaged in 2004. MEGAPIE is a first decisive step to realize a liquid metal spallation target in Europe. This report is giving an overview of the MEGAPIE-TEST Project, the overall work plan, and preliminary results from the design support and validation, which form an important basis for the project. (authors)

  10. Three years of cross-section measurements of (n,xn threshold reactions at TSL Uppsala and NPI Řež

    Directory of Open Access Journals (Sweden)

    Majerle M.

    2010-10-01

    Full Text Available We use (n,xn threshold reactions in various materials to measure high energy neutron flux from spallation reactions. Unfortunately, no experimental cross-section data exist for reactions with x higher than four and neutron energies over ∼  40  MeV. With the support from EFNUDAT we performed seven successful (n,xn cross-section measurements in two campaigns exploiting the quasi-monoenergetic neutron source at The Svedberg Laboratory in Uppsala, Sweden. Neutron energies from the 7Li(p, n7Be based source were in the region 22 to 94 MeV. We carried out additional four irradiations with neutron energies from 17 up to 34 MeV using the quasi-monoenergetic neutron source of the Nuclear Physics Institute in Řež. We studied Al, Au, Bi, I, In, and Ta materials. Although we used different neutron sources, gamma detectors and foil geometries, we obtained consistent results. We observed good agreement with the data in EXFOR, so we believe we have understood and solved all possible sources of uncertainties.

  11. Non-equilibrium effects in high temperature chemical reactions

    Science.gov (United States)

    Johnson, Richard E.

    1987-01-01

    Reaction rate data were collected for chemical reactions occurring at high temperatures during reentry of space vehicles. The principle of detailed balancing is used in modeling kinetics of chemical reactions at high temperatures. Although this principle does not hold for certain transient or incubation times in the initial phase of the reaction, it does seem to be valid for the rates of internal energy transitions that occur within molecules and atoms. That is, for every rate of transition within the internal energy states of atoms or molecules, there is an inverse rate that is related through an equilibrium expression involving the energy difference of the transition.

  12. Los Alamos pulsed spallation neutron source target systems - present and future

    International Nuclear Information System (INIS)

    Russell, G.J.; Daemen, L.L.; Pitcher, E.J.; Brun, T.O.; Hjelm, R.P. Jr.

    1993-01-01

    For the past 16 yr, spallation target-system designers have devoted much time and effort to the design and optimization of pulsed spallation neutron sources. Many concepts have been proposed, but, in practice, only one has been implemented horizontal beam insertion with moderators in wing geometry i.e., until we introduced the innovative split-target/flux-trap-moderator design with a composite reflector shield at the Manuel Lujan, Jr., Neutron Scattering Center (LANSCE). The LANSCE target system design is now considered a classic by spallation target system designers worldwide. LANSCE, a state-of-the-art pulsed spallation neutron source for materials science and nuclear physics research, uses 800-MeV protons from the Clinton P. Anderson Meson Physics Facility. These protons are fed into the proton storage ring to be compressed to 250-ns pulses before being delivered to LANSCE at 20 Hz. LANSCE produces the highest peak neutron flux of any pulsed spallation neutron source in the world

  13. Radiation damage for the spallation target of ADS

    International Nuclear Information System (INIS)

    Fan Sheng; Ye Yanlin; Xu Chuncheng; Chen Tao; Sobolevsky, N.M.

    2000-01-01

    By using SHIELD codes system, the authors investigate the radiation damage, such as radiation damage cross section, displacement atom cross section and the rate of displacement atom, gas production cross section, the rate of gas production and the ratio, R, of the helium and displacement production rates in target, container window and spallation neutron source materials as W and Pb induced from intermediate energy proton and neutron incident. And the study of radiation damage in the thick Pb target with long 60 cm, radius 20 cm is presented

  14. High energy hadron-nucleus collision

    International Nuclear Information System (INIS)

    Takagi, Fujio

    1983-02-01

    This is a lecture note concerning high energy hadron-nucleus collision. The lecture gives the inelastic total cross section and the Glanber approximate multiple scattering formula at first. The mechanism of nuclear spallation is described in a cylindrical image. The multiplicity, the one particle distribution and the time-space structure of particle production are discussed. Various models are presented. The attenuation of forward particles and the structure of hadrons are discussed for each model. The atomic number (A) dependence of the production of large transverse momentum particles and jet, and the A dependence of charged multiplicity are presented. The backward production of particles and many body correlation are discussed. Lepton pair production and the initial interaction of constituents, collective interaction, multi quark state and phase transition are described. (Kato, T.)

  15. Dynamics of anion-molecule reactions at low energy

    International Nuclear Information System (INIS)

    Mikosch, J.

    2007-11-01

    Anion-molecule reactions must find their way through deeply bound entrance and exit channel complexes separated by a central barrier. This results in low reaction rates and rich dynamics since direct pathways compete with the formation of transient intermediates. In this thesis we examine the probability of proton transfer to a small anion and transient lifetimes of a thermoneutral bimolecular nucleophilic substitution (S N 2) reaction at well defined variable temperature down to 8 Kelvin in a multipole trap. The observed strong inverse temperature dependence is attributed to the deficit of available quantum states in the entrance channel at decreasing temperature. Furthermore we investigate scattering dynamics of S N 2 reactions at defined relative energy between 0.4 and 10 eV by crossed beam slice imaging. A weakly exothermic reaction with high central barrier proceeds via an indirect, complex-mediated mechanism at low relative energies featuring high internal product excitation in excellent quantitative agreement with a statistical model. In contrast, direct backward scattering prevails for higher energies with product velocities close to the kinematical cutoff. For a strongly exothermic reaction, competing S N 2-, dihalide- and proton transfer-channels are explored which proceed by complex mediation for low energy and various rebound-, grazing- and collision induced bond rupture-mechanisms at higher energy. From our data and a collaboration with theory we identify a new indirect roundabout S N 2 mechanism involving CH 3 -rotation. (orig.)

  16. Dynamics of anion-molecule reactions at low energy

    Energy Technology Data Exchange (ETDEWEB)

    Mikosch, J.

    2007-11-15

    Anion-molecule reactions must find their way through deeply bound entrance and exit channel complexes separated by a central barrier. This results in low reaction rates and rich dynamics since direct pathways compete with the formation of transient intermediates. In this thesis we examine the probability of proton transfer to a small anion and transient lifetimes of a thermoneutral bimolecular nucleophilic substitution (S{sub N}2) reaction at well defined variable temperature down to 8 Kelvin in a multipole trap. The observed strong inverse temperature dependence is attributed to the deficit of available quantum states in the entrance channel at decreasing temperature. Furthermore we investigate scattering dynamics of S{sub N}2 reactions at defined relative energy between 0.4 and 10 eV by crossed beam slice imaging. A weakly exothermic reaction with high central barrier proceeds via an indirect, complex-mediated mechanism at low relative energies featuring high internal product excitation in excellent quantitative agreement with a statistical model. In contrast, direct backward scattering prevails for higher energies with product velocities close to the kinematical cutoff. For a strongly exothermic reaction, competing S{sub N}2-, dihalide- and proton transfer-channels are explored which proceed by complex mediation for low energy and various rebound-, grazing- and collision induced bond rupture-mechanisms at higher energy. From our data and a collaboration with theory we identify a new indirect roundabout S{sub N}2 mechanism involving CH{sub 3}-rotation. (orig.)

  17. Numerical Simulations of Thermo-Mechanical Processes during Thermal Spallation Drilling for Geothermal Reservoirs

    Science.gov (United States)

    Vogler, D.; Walsh, S. D. C.; Rudolf von Rohr, P.; Saar, M. O.

    2017-12-01

    Drilling expenses constitute a significant share of the upfront capital costs and thereby the associated risks of geothermal energy production. This is especially true for deep boreholes, as drilling costs per meter increase significantly with depth. Thermal spallation drilling is a relatively new drilling technique, particularly suited to the hard crystalline (e.g., basement) rocks in which many deep geothermal resources are located. The method uses a hot jet-flame to rapidly heat the rock surface, which leads to large temperature gradients in the rock. These temperature gradients cause localized thermal stresses that, in combination with the in situ stress field, lead to the formation and ejection of spalls. These spalls are then transported out of the borehole with the drilling mud. Thermal spallation not only in principle enables much faster rates of penetration than traditional rotary drilling, but is also contact-less, which significantly reduces the long tripping times associated with conventional rotary head drilling. We present numerical simulations investigating the influence of rock heterogeneities on the thermal spallation process. Special emphasis is put on different mineral compositions, stress regimes, and heat sources.

  18. Low energy ion-molecule reactions

    Energy Technology Data Exchange (ETDEWEB)

    Farrar, J.M. [Univ. of Rochester, NY (United States)

    1993-12-01

    This project is concerned with elucidating the dynamics of elementary ion-molecule reactions at collision energies near and below 1 eV. From measurements of the angular and energy distributions of the reaction products, one can infer intimathe details about the nature of collisions leading to chemical reaction, the geometries and lifetimes of intermediate complexes that govern the reaction dynamics, and the collision energy dependence of these dynamical features. The author employs crossed-beam low energy mass spectrometry technology developed over the last several years, with the focus of current research on proton transfer and hydrogen atom transfer reactions of te O{sup {minus}} ion with species such as HF, H{sub 2}O, and NH{sub 3}.

  19. Spallation integral experiment analysis by high energy nucleon-meson transport code

    Energy Technology Data Exchange (ETDEWEB)

    Takada, Hiroshi; Meigo, Shin-ichiro; Sasa, Toshinobu; Fukahori, Tokio [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment; Yoshizawa, Nobuaki; Furihata, Shiori; Belyakov-Bodin, V.I.; Krupny, G.I.; Titarenko, Y.E.

    1997-03-01

    Reaction rate distributions were measured with various activation detectors on the cylindrical surface of the thick tungsten target of 20 cm in diameter and 60 cm in length bombarded with the 0.895 and 1.21 GeV protons. The experimental results were analyzed with the Monte Carlo simulation code systems of NMTC/JAERI-MCNP-4A, LAHET and HERMES. It is confirmed that those code systems can represent the reaction rate distributions with the C/E ratio of 0.6 to 1.4 at the positions up to 30 cm from beam incident surface. (author)

  20. The US spallation neutron source (SNS) project

    International Nuclear Information System (INIS)

    Alonso, J.R.

    1999-01-01

    The SNS is a 1 MW pulsed spallation neutron source that will be sited at Oak Ridge. It will consist of a high-current, normal-conducting linac accelerating an H - beam to 1 GeV, an accumulator ring which compresses each 1 ms linac pulse into a 600 ns bunch which is then extracted in a single turn onto a liquid mercury target. Neutron pulses emerge at a 60 Hz rate from the two ambient, and two cryogenic moderators. Eighteen beam ports surrounding the target station are available for neutron-scattering instrumentation. Funds for ten instruments are included in the construction project; these instruments will provide basic measurement capability for the many and varied research activities at the SNS facility. The new spallation source is being built by a consortium of laboratories; the partners are LBNL, LANL, BNL, ANL and ORNL. The breadth and depth of experience and resources brought by such a wide-spread team offers very significant advantages. Construction will start in October of 1998, operation will begin in October, 2005. (J.P.N.)

  1. Tensile property changes of metals and irradiated to low doses with fission, fusion and spallation neutrons

    International Nuclear Information System (INIS)

    Heinisch, H.L.; Hamilton, M.L.; Sommer, W.F.; Ferguson, P.D.

    1992-01-01

    The objective of this work is to investigate the effects of the neutron energy spectrum in low dose irradiations on the microstructures and mechanical properties of metals. Radiation effects due to low doses of spallation neutrons are compared directly to those produced by fission and fusion neutrons. Yield stress changes of pure Cu, alumina-dispersion-strengthened Cu and AISI 316 stainless steel irradiated at 36-55 C in the Los Alamos Spallation Radiation Effects Facility (LASREF) are compared with earlier results of irradiations at 90 C using 14 MeV D-T fusion neutrons at the Rotating Target Neutron Source and fission reactor neutrons in the Omega West Reactor. At doses up to 0.04 displacements per atom (dpa), the yield stress changes due to the three quite different neutron spectra correlate well on the basis of dpa in the stainless steel and the Cu alloy. However, in pure Cu, the measured yield stress changes due to spallation neutrons were anomalously small and should be verified by additional irradiations. With the exception of pure Cu, the low dose, low temperature experiments reveal no fundamental differences in radiation hardening by fission, fusion or spallation neutrons when compared on the basis of dpa

  2. Improved design of proton source and low energy beam transport line for European Spallation Source

    Energy Technology Data Exchange (ETDEWEB)

    Neri, L., E-mail: neri@lns.infn.it; Celona, L.; Gammino, S.; Mascali, D.; Castro, G.; Ciavola, G. [Laboratori Nazionali del Sud, Istituto Nazionale di Fisica Nucleare, Via S. Sofia 62, 95123 Catania (Italy); Torrisi, G. [Laboratori Nazionali del Sud, Istituto Nazionale di Fisica Nucleare, Via S. Sofia 62, 95123 Catania (Italy); Dipartimento di Ingegneria dell’Informazione, delle Infrastrutture e dell’Energia Sostenibile, Università Mediterranea di Reggio Calabria, Via Graziella, 89122 Reggio Calabria (Italy); Cheymol, B.; Ponton, A. [European Spallation Source ESS AB, Lund (Sweden); Galatà, A. [Laboratori Nazionali di Legnaro, Istituto Nazionale di Fisica Nucleare, Viale dell' università 2, 35020 Legnaro (Italy); Patti, G. [Laboratori Nazionali del Sud, Istituto Nazionale di Fisica Nucleare, Via S. Sofia 62, 95123 Catania (Italy); Laboratori Nazionali di Legnaro, Istituto Nazionale di Fisica Nucleare, Viale dell' università 2, 35020 Legnaro (Italy); Gozzo, A.; Lega, L. [Laboratori Nazionali del Sud, Istituto Nazionale di Fisica Nucleare, Via S. Sofia 62, 95123 Catania (Italy); Dipartimento di Ingegneria Informatica e delle Telecomunicazioni, Università degli Studi di Catania, Viale Andrea Doria 6, 95123 Catania (Italy)

    2014-02-15

    The design update of the European Spallation Source (ESS) accelerator is almost complete and the construction of the prototype of the microwave discharge ion source able to provide a proton beam current larger than 70 mA to the 3.6 MeV Radio Frequency Quadrupole (RFQ) started. The source named PS-ESS (Proton Source for ESS) was designed with a flexible magnetic system and an extraction system able to merge conservative solutions with significant advances. The ESS injector has taken advantage of recent theoretical updates and new plasma diagnostics tools developed at INFN-LNS (Laboratori Nazionali del Sud, Istituto Nazionale di Fisica Nucleare). The design strategy considers the PS-ESS and the low energy beam transport line as a whole, where the proton beam behaves like an almost neutralized non-thermalized plasma. Innovative solutions have been used as hereinafter described. Thermo-mechanical optimization has been performed to withstand the chopped beam and the misaligned focused beam over the RFQ input collimator; the results are reported here.

  3. Measurement of cross sections for the scattering of neutrons in the energy range from 2 MeV to 4 MeV with the 15N(p,n) reaction as neutron source

    International Nuclear Information System (INIS)

    Poenitz, Erik

    2010-01-01

    In future nuclear facilities, the materials lead and bismuth can play a more important role than in today's nuclear reactors. Reliable cross section data are required for the design of those facilities. In particular the neutron transport in the lead spallation target of an Accelerator-Driven Subcritical Reactor strongly depends on the inelastic neutron scattering cross sections in the energy region from 0.5 MeV to 6 MeV. In the recent 20 years, elastic and inelastic neutron scattering cross sections were measured with high precision for a variety of elements at the PTB time-of-flight spectrometer. The D(d,n) reaction was primarily used for the production of neutrons. Because of the Q value of the reaction and the available deuteron energies, neutrons in the energy range from 6 MeV to 16 MeV can be produced. For the cross section measurement at lower energies, however, another neutron producing reaction is required. The 15 N(p,n) 15 O reaction was chosen, as it allows the production of monoenergetic neutrons with up to 5.7MeV energy. In this work, the 15 N(p,n) reaction was studied with focus on the suitability as a source for monoenergetic neutrons in scattering experiments. This includes the measurement of differential cross sections for the neutron producing reaction and the choice of optimum target conditions. Differential elastic and inelastic neutron scattering cross sections were measured for lead at four energies in the region from 2 MeV to 4 MeV incident neutron energy using the time-of-flight technique. A lead sample with natural isotopic composition was used. NE213 liquid scintillation detectors with well-known detection efficiencies were used for the detection of the scattered neutrons. Angle-integrated cross sections were determined by a Legendre polynomial expansion using least-squares methods. Additionally, measurements were carried out for isotopically pure 209 Bi and 181 Ta samples at 4 MeV incident neutron energy. Results are compared with other

  4. Generation and scaling behaviour of high-energy pions in relativistic heavy ion reactions

    International Nuclear Information System (INIS)

    Riess, F.

    1979-12-01

    Calculations with the help of a collision approximation as carried out in this study, are certainly linked with many uncertainties. The different forms of pulse distributions and cross sections used cover however such a broad region of possibilities, that even detailed calculations will not give any results essentially deviating from those obtained here. The various assumptions and statements could be relatively easily investigated using the collision approximation. Hence the above-mentioned aim, to pick out the principal information from the statement is achieved. It was shown that taking the two assumptions - nucleon-nucleon collisions only and - consideration of a cluster effect, in both cases the experimental results for a given reaction can be well reproduced as long as one only regards one projectile energy. It is important in the first case that the pulse distribution in the region of 0,5 to 1 GeV/c contains sufficiently large components - a simple Gauss distribution with a 'normal' parameter from nuclean physics is not sufficient here. The cluster statement provides the high-energy pions through the changed kinematics, compared to pure nucleon-nucleon collisions, and through the greater energy provided by a cluster in the reaction. (orig./HSI) [de

  5. Advanced spallation neutron sources for condensed matter research

    International Nuclear Information System (INIS)

    Lovesey, S.W.; Stirling, G.C.

    1984-03-01

    Advanced spallation neutron sources afford significant advantages over existing high flux reactors. The effective flux is much greater than that currently available with reactor sources. A ten-fold increase in neutron flux will be a major benefit to a wide range of condensed matter studies, and it will realise important experiments that are marginal at reactor sources. Moreover, the high intensity of epithermal neutrons open new vistas in studies of electronic states and molecular vibrations. (author)

  6. Nuclear waste transmutation

    International Nuclear Information System (INIS)

    Leray, S.

    1995-01-01

    Accelerators can play a role in the disposal of long-lived radioactive waste: an alternative to the storage in deep underground repositories might transmuting long-lived elements into stable or short-lived ones in subcritical systems driven by spallation neutrons. These neutrons would be produced by a high intensity, intermediate energy proton accelerator irradiating a heavy target. Similar systems have also been proposed to produce energy with a minimized waste inventory. Since a good knowledge of the spallation process is essential for designing and optimizing the target-blanket assembly, new programmes aimed at studying spallation reactions are in progress. (author). 6 figs

  7. Safety-technical lay-out of the operational environment of a high-power spallation target system of the megawatt class with mercury as target material

    International Nuclear Information System (INIS)

    Butzek, M.

    2005-06-01

    of the neutron guide system. Due to the high amount of safety relevant handling procedures, concepts for time efficient and safe handling of the major components have been developed. Based on the concepts shown in this thesis, construction and operation of a high power spallation source of the described kind seem to be feasible considering safety and costs. (orig.)

  8. Status of SINQ, the only MW spallation neutron source-highlighting target development and industrial applications

    International Nuclear Information System (INIS)

    Wagner, Werner; Dai, Yong; Glasbrenner, Heike; Grosse, Mirco; Lehmann, Eberhard

    2006-01-01

    SINQ is a continuous spallation neutron source, driven by PSI's 590 MeV proton accelerator. Receiving a stable proton current of 1.3 mA, SINQ is the presently most powerful accelerator-driven facility worldwide. Besides the primary designation of SINQ to serve as user facility for neutron scattering and neutron imaging, PSI seeks to play a leading role in the development of the facility, focusing on spallation targets and materials research for high-dose radiation environments. Accompanying these activities, SINQ has established several projects serving a more general, profound development towards high-power spallation targets: the most prominent ones being SINQ Target Irradiation Program (STIP) and megawatt pilot experiment for a liquid metal target (MEGAPIE), complemented by LiSoR and VIMOS. Within the user program, SINQ is aspiring to attract an appropriate contingent of industrial applications. The paper highlights the potential for industrial applications by means of selected examples from strain mapping and neutron imaging

  9. The two-proton halo nucleus {sup 17}Ne studied in high-energy nuclear breakup reactions

    Energy Technology Data Exchange (ETDEWEB)

    Wamers, Felix [EMMI, GSI, Darmstadt (Germany); FIAS, Frankfurt (Germany); IKP, TU Darmstadt, Darmstadt (Germany); GSI, Darmstadt (Germany); Marganiec, Justyna [IKP, TU Darmstadt, Darmstadt (Germany); EMMI, GSI, Darmstadt (Germany); GSI, Darmstadt (Germany); Aumann, Thomas [IKP, TU Darmstadt, Darmstadt (Germany); GSI, Darmstadt (Germany); Bertulani, Carlos [Texas A and M University-Commerce, Commerce (United States); Chulkov, Leonid [GSI, Darmstadt (Germany); NRC Kurchatov Institute, Moscow (Russian Federation); Heil, Michael; Simon, Haik [GSI, Darmstadt (Germany); Plag, Ralf [GSI, Darmstadt (Germany); Goethe Universitaet, Frankfurt (Germany); Savran, Deniz [EMMI, GSI, Darmstadt (Germany); FIAS, Frankfurt (Germany); Collaboration: R3B-Collaboration

    2014-07-01

    We report on exclusive measurements of nuclear breakup reactions of highly-energetic (500 MeV) unstable {sup 17}Ne beams impinging on light targets in an experiment at the R{sup 3}B-LAND complete-kinematics reaction setup at GSI. Focusing on the properties of beam-like {sup 15}O-p (={sup 16}F) systems produced in one-proton-removal reactions, we are presenting a comprehensive analysis of the s-/d-wave configuration mixing of the {sup 17}Ne valence-proton pair that is used to quantify its halo-nature. The results include the {sup 15}O-p relative-energy spectrum, {sup 16}F momentum distributions, and their corresponding momentum profile.

  10. Tool for the study of matter - the spallation neutron source. Werkzeug zur Erforschung der Materie - die Spallations-Neutronenquelle

    Energy Technology Data Exchange (ETDEWEB)

    1983-01-01

    It deals with the optimal use of a whole series of matter penetrating radiation types at the construction of a spallation neutron source which the Kernforschungsanlage Juelich will realize in agreement with its associated. This new big science device for the fundamental research in the Federal Republic of Germany shall as the most modern and intense source of neutrons, protons, pions, muons, and neutrinos permits to proceed in the fields of solid state physics, chemistry, molecular biology, intermediate-energy nuclear physics, radiochemistry and radiopharmacology, medicine, and materials science to virgin territory and to provide top research. All interested German groups of researchers and also scientists of foreign countries shall be able to work with this directive big science device.

  11. Studies of high energy hadron-hadron reactions

    International Nuclear Information System (INIS)

    Maansson, O.

    1982-01-01

    The first part of this thesis concerns the possibility of obtaining a quantity that reveals more of the primary scattering of partons, than the single particle spectra for high-p(sub)T reactions. K -K is shown to be such a quantity for 90degree scattering. A p(sub)T-dependence of P(sub)t(sup)-5.4 is data from FNAL and ISR. A model for low-p(sub)T baryon production is presented. This one-dimensional string model gives longitudinal single particle spectra in good agreement with exp. data. A model for polarization of inclusively produced hyperons is presented. A baryon is pictured as a Y-shaped string with quarks at the ends. One of the quarks is kicked out in the reaction, leading to a basically one-dim. string system. The motion of the string junction is shown to be important for the understanding of polarization phenomena. Lowest order QCD is studied with respect to color factors in the production amplitude in order to find final string configurations in high-p(sub)T events. The basis for a Monte Carlo program for complete high-p(sub)T events is discussed. (author)

  12. Results from the TARC experiment: spallation neutron phenomenology in lead and neutron-driven nuclear transmutation by adiabatic resonance crossing

    Science.gov (United States)

    Abánades, A.; Aleixandre, J.; Andriamonje, S.; Angelopoulos, A.; Apostolakis, A.; Arnould, H.; Belle, E.; Bompas, C. A.; Brozzi, D.; Bueno, J.; Buono, S.; Carminati, F.; Casagrande, F.; Cennini, P.; Collar, J. I.; Cerro, E.; Del Moral, R.; Díez, S.; Dumps, L.; Eleftheriadis, C.; Embid, M.; Fernández, R.; Gálvez, J.; García, J.; Gelès, C.; Giorni, A.; González, E.; González, O.; Goulas, I.; Heuer, D.; Hussonnois, M.; Kadi, Y.; Karaiskos, P.; Kitis, G.; Klapisch, R.; Kokkas, P.; Lacoste, V.; Le Naour, C.; López, C.; Loiseaux, J. M.; Martínez-Val, J. M.; Méplan, O.; Nifenecker, H.; Oropesa, J.; Papadopoulos, I.; Pavlopoulos, P.; Pérez-Enciso, E.; Pérez-Navarro, A.; Perlado, M.; Placci, A.; Poza, M.; Revol, J.-P.; Rubbia, C.; Rubio, J. A.; Sakelliou, L.; Saldaña, F.; Savvidis, E.; Schussler, F.; Sirvent, C.; Tamarit, J.; Trubert, D.; Tzima, A.; Viano, J. B.; Vieira, S.; Vlachoudis, V.; Zioutas, K.

    2002-02-01

    We summarize here the results of the TARC experiment whose main purpose is to demonstrate the possibility of using Adiabatic Resonance Crossing (ARC) to destroy efficiently Long-Lived Fission Fragments (LLFFs) in accelerator-driven systems and to validate a new simulation developed in the framework of the Energy Amplifier programme. An experimental set-up was installed in a CERN PS proton beam line to study how neutrons produced by spallation at relatively high energy ( E n⩾1 MeV) slow down quasi-adiabatically with almost flat isolethargic energy distribution and reach the capture resonance energy of an element to be transmuted where they will have a high probability of being captured. Precision measurements of energy and space distributions of spallation neutrons (using 2.5 and 3.5 GeV/ c protons) slowing down in a 3.3 m×3.3 m×3 m lead volume and of neutron capture rates on LLFFs 99Tc, 129I, and several other elements were performed. An appropriate formalism and appropriate computational tools necessary for the analysis and understanding of the data were developed and validated in detail. Our direct experimental observation of ARC demonstrates the possibility to destroy, in a parasitic mode, outside the Energy Amplifier core, large amounts of 99Tc or 129I at a rate exceeding the production rate, thereby making it practical to reduce correspondingly the existing stockpile of LLFFs. In addition, TARC opens up new possibilities for radioactive isotope production as an alternative to nuclear reactors, in particular for medical applications, as well as new possibilities for neutron research and industrial applications.

  13. CFD studies on thermal hydraulics of spallation targets

    International Nuclear Information System (INIS)

    Tak, N.I.; Batta, A.; Cheng, X.

    2005-01-01

    Full text of publication follows: Due to the fast advances in computer hardware as well as software in recent years, more and more interests have been aroused to use computational fluid dynamics (CFD) technology in nuclear engineering and designs. During recent many years, Forschungszentrum Karlsruhe (FZK) has been actively involved in the thermal hydraulic analysis and design of spallation targets. To understand the thermal hydraulic behaviors of spallation targets very detailed simulations are necessary because of their complex geometries, complicated boundary conditions such as spallation heat distributions, and very strict design limits. A CFD simulation is believed to be the best for this purpose even though the validation of CFD codes are not perfectly completed yet in specific topics like liquid metal heat transfer. The research activities on three spallation targets (i.e., MEGAPIE, TRADE, and XADS targets) are currently very active in Europe in order to consolidate the European ADS road-map. In the thermal hydraulics point of view, two kinds of the research activities, i.e., (1) numerical design and (2) experimental work, are required to achieve the objectives of these targets. It should be noted that CFD studies play important role on both kinds of two activities. A preliminary design of a target can be achieved by sophisticated CFD analysis and pre-and-post analyses of an experimental work using a CFD code help the design of the test section of the experiment as well as the analysis of the experimental results. The present paper gives an overview about the recent CFD studies relating to thermal hydraulics of the spallation targets recently involved in FZK. It covers numerical design studies as well as CFD studies to support experimental works. The CFX code has been adopted for the studies. Main recent results for the selected examples performed by FZK are presented and discussed with their specific lessons learned. (authors)

  14. Cross-sections of residual nuclei from deuteron irradiation of thin thorium target at energy 7 GeV

    Directory of Open Access Journals (Sweden)

    Vespalec Radek

    2017-01-01

    Full Text Available The residual nuclei yields are of great importance for the estimation of basic radiation-technology characteristics (like a total target activity, production of long-lived nuclides etc. of accelerator driven systems planned for transmutation of spent nuclear fuel and for a design of radioisotopes production facilities. Experimental data are also essential for validation of nuclear codes describing various stages of a spallation reaction. Therefore, the main aim of this work is to add new experimental data in energy region of relativistic deuterons, as similar data are missing in nuclear databases. The sample made of thin natural thorium foil was irradiated at JINR Nuclotron accelerator with a deuteron beam of the total kinetic energy 7 GeV. Integral number of deuterons was determined with the use of aluminum activation detectors. Products of deuteron induced spallation reaction were qualified and quantified by means of gamma-ray spectroscopy method. Several important spectroscopic corrections were applied to obtain results of high accuracy. Experimental cumulative and independent cross-sections were determined for more than 80 isotopes including meta-stable isomers. The total uncertainty of results rarely exceeded 9%. Experimental results were compared with MCNP6.1 Monte-Carlo code predictions. Generally, experimental and calculated cross-sections are in a reasonably good agreement, with the exception of a few light isotopes in a fragmentation region, where the calculations are highly under-estimated. Measured data will be useful for future development of high-energy nuclear codes. After completion, final data will be added into the EXFOR database.

  15. Reversible aqueous zinc/manganese oxide energy storage from conversion reactions

    Energy Technology Data Exchange (ETDEWEB)

    Pan, Huilin; Shao, Yuyan; Yan, Pengfei; Cheng, Yingwen; Han, Kee Sung; Nie, Zimin; Wang, Chongmin; Yang, Jihui; Li, Xiaolin; Bhattacharya, Priyanka; Mueller, Karl T.; Liu, Jun

    2016-04-18

    Rechargeable aqueous batteries are attracting growing interest for energy storage due to their low cost and high safety. Fundamental understanding of highly reversible aqueous reactions is critical for building high-performance batteries. Herein, we studied the reversibility of Zn/MnO2 battery chemistry in mild aqueous MnSO4 electrolytes. α-MnO2 nanofibers were used as a high performance cathode. Our study provides good evidence for a conversion reaction mechanism through reversible formation of short nanorods and nanoparticle aggregates. This reversible conversion reaction provides an operating voltage of 1.44 V, high capacity of 285 mAh g-1, excellent rate and capacity retention of 92% after 5000 cycles. Zn metal anode also shows high reversibility in the mild aqueous MnSO4 electrolytes. The highly reversible and stable chemistries in aqueous Zn/MnO2 batteries open new opportunity for energy storage technologies with potentially high energy density, high safety, and low cost.

  16. Towards the construction of the European spallation source–The ...

    Indian Academy of Sciences (India)

    The possible realization of the European spallation source has been a long and winding story. However, thanks to the conjunction of a number of events it now looks highly probable that in 2008 there will indeed be a decision on the site and on a funding partnership of European countries who will together build and ...

  17. Dissipative effects in fission investigated with proton-on-lead reactions

    Directory of Open Access Journals (Sweden)

    Rodríguez-Sánchez J. L.

    2016-01-01

    Full Text Available The complete kinematic measurement of the two fission fragments permitted us to investigate dissipative effects at large deformations, between the saddle-point and the corresponding scission configurations. Up to now, this kind of study has only been performed with fusionfission reactions using a limited number of observables, such as the mass distribution of the fission fragments or the neutron multiplicities. However, the large angular momenta gained by the compound nucleus could affect the conclusions drawn from such experiments. In this work, the use of spallation reactions, where the fissioning systems are produced with low angular momentum, small deformations and high excitation energies, favors the study of dissipation, and allowed us to define new observables, such as postscission neutron multiplicities and the neutron excess of the final fission fragments as a function of the atomic number of the fissioning system. These new observables are used to investigate the dissipation at large deformations.

  18. New science at the European Spallation Source

    Energy Technology Data Exchange (ETDEWEB)

    Finney, J L [University Coll., London (United Kingdom). Dept. of Physics and Astronomy

    1996-05-01

    The European Spallation Source is a trans-European project aimed at the ultimate construction of a next-generation pulsed spallation neutron source that will deliver 30 times the beam power of ISIS. The reference design for the proposed source has been set, and work is in progress to develop an updated scientific case for the construction of the source early in the next century. Together with improvements in instrumentation, effective flux gains of over two orders of magnitude are likely in some areas, opening up major new opportunities for the exploitation of neutron studies in fundamental, strategic, and applied science. (author)

  19. New findings on the onset of thermal disassembly in spallation reactions

    International Nuclear Information System (INIS)

    Napolitani, P.

    2004-09-01

    Thermal multifragmentation is the process of multi body disassembly of a hot nucleus when the excitation is almost purely thermal i.e. dynamical effects like compression (characteristic of ion-ion collisions at Fermi energy) are negligible. Suited reactions are proton induced collision or ion-ion abrasion at relativistic incident energy. Thus we measured four systems at FRS (Fragment separator, GSI, Darmstadt) in inverse kinematics: Fe 56 +p, Fe 56 +Ti(nat), Xe 136 +p, Xe 136 +Ti(nat) a 1 A*GeV. The inverse kinematics allows to observe all particles without any threshold in energy. This is a great advantage compared to experiments in direct kinematics, because only in inverse kinematics it is possible to obtain complete velocity spectra (without a hole for low velocities) for fully identified isotopes. The complex shape of the velocity spectra allows to identify the different deexcitation channels and it clearly shows the transition from a chaotic-dominated process (Gaussian cloud in velocity space) to a direct Coulomb- (or eventually expansion-) dominated process (shell of a sphere in velocity space). Different possible descriptions of the reaction process are discussed, based either on asymmetric fission or multifragmentation. The resulting physical picture is especially interesting for the Fe 56 +p, and Xe 136 +p systems: proton induced collisions could result in the split of the system in two or more fragments due to a fast break-up process. In this case, the configuration of the break-up partition is very asymmetric. The discussion will be extended to other characteristics, like the restoring of nuclear structure features in the isotopic production and the temperature dependence of the isotopic composition of the residues. (author)

  20. The very low angle detector for high-energy inelastic neutron scattering on the VESUVIO spectrometer

    International Nuclear Information System (INIS)

    Perelli Cippo, E.; Gorini, G.; Tardocchi, M.; Pietropaolo, A.; Andreani, C.; Senesi, R.; Rhodes, N.J.; Schooneveld, E.M.

    2008-01-01

    The Very Low Angle Detector (VLAD) bank has been installed on the VESUVIO spectrometer at the ISIS spallation neutron source. The new device allows for high-energy inelastic neutron scattering measurements, at energies above 1 eV, maintaining the wave vector transfer lower than 10A -1 . This opens a still unexplored region of the kinematical (q,ω) space, enabling new and challenging experimental investigations in condensed matter. This paper describes the main instrumental features of the VLAD device, including instrument design, detector response, and calibration procedure

  1. The very low angle detector for high-energy inelastic neutron scattering on the VESUVIO spectrometer

    Science.gov (United States)

    Perelli Cippo, E.; Gorini, G.; Tardocchi, M.; Pietropaolo, A.; Andreani, C.; Senesi, R.; Rhodes, N. J.; Schooneveld, E. M.

    2008-05-01

    The Very Low Angle Detector (VLAD) bank has been installed on the VESUVIO spectrometer at the ISIS spallation neutron source. The new device allows for high-energy inelastic neutron scattering measurements, at energies above 1 eV, maintaining the wave vector transfer lower than 10Å-1. This opens a still unexplored region of the kinematical (q, ω) space, enabling new and challenging experimental investigations in condensed matter. This paper describes the main instrumental features of the VLAD device, including instrument design, detector response, and calibration procedure.

  2. The spallation neutron source: New opportunities

    Indian Academy of Sciences (India)

    The spallation neutron source (SNS) facility became operational in the spring of ... the opportunity to develop science and instrumentation programs which take ... in telecommunications, manufacturing, transportation, information technology, ...

  3. A target-moderator-reflector concept of the JAERI 5 MW pulsed spallation neutron source

    International Nuclear Information System (INIS)

    Watanabe, Noboru; Teshigawara, Makoto; Aizawa, Kazuya; Suzuki, Jyunichi; Oyama, Yukio

    1998-03-01

    In Japan Atomic Energy Research Institute the construction of a 5 MW (short) pulsed spallation neutron source is under planning using a projected high power superconducting proton (or H - ) linac of 8 MW in total beam power. In the present paper we report our consideration on target-moderator-reflector concept, based on the layout of the tentative neutron instruments for the assumed neutron scattering experiments in future. The choice of cold neutron moderators for high resolution and high intensity experiments, thermal and epithermal neutron moderators for high resolution uses was discussed and a reference layout of target-moderator-reflector system was proposed for detailed neutronic calculation and optimization. The proposed system was designed like that it can provide, at least, 30 beam lines for more than 40 instruments. (author)

  4. Experimental setup and procedure for the measurement of the {sup 7}Be(n,α)α reaction at n-TOF

    Energy Technology Data Exchange (ETDEWEB)

    Cosentino, L. [INFN Laboratori Nazionali del Sud, Catania (Italy); Musumarra, A. [INFN Laboratori Nazionali del Sud, Catania (Italy); Dipartimento di Fisica e Astronomia DFA, Università di Catania (Italy); Barbagallo, M. [INFN Sezione di Bari (Italy); Pappalardo, A. [INFN Laboratori Nazionali del Sud, Catania (Italy); Colonna, N.; Damone, L. [INFN Sezione di Bari (Italy); Piscopo, M. [INFN Laboratori Nazionali del Sud, Catania (Italy); Finocchiaro, P., E-mail: FINOCCHIARO@LNS.INFN.IT [INFN Laboratori Nazionali del Sud, Catania (Italy); Maugeri, E.; Heinitz, S.; Schumann, D.; Dressler, R.; Kivel, N. [Paul Scherrer Institut, Nuclear Energy and Safety Research Department, 5232 Villigen (Switzerland); Aberle, O. [CERN, Geneva (Switzerland); Andrzejewski, J. [Uniwersytet Łódzki, Lodz (Poland); Audouin, L. [Institut de Physique Nucléaire, CNRS-IN2P3, Univ. Paris-Sud, Université Paris-Saclay, 91406 Orsay Cedex (France); Ayranov, M. [European Commission, DG-Energy (Luxembourg); Bacak, M. [Atominstitut der Österreichischen Universitäten, Technische Universität Wien (Austria); Barros, S. [C2TN-Instituto Superior Tecníco, Universidade de Lisboa (Portugal); Balibrea-Correa, J. [Centro de Investigaciones Energeticas Medioambientales y Tecnológicas (CIEMAT), Madrid (Spain); and others

    2016-09-11

    The newly built second experimental area EAR2 of the n-TOF spallation neutron source at CERN allows to perform (n, charged particles) experiments on short-lived highly radioactive targets. This paper describes a detection apparatus and the experimental procedure for the determination of the cross-section of the {sup 7}Be(n,α)α reaction, which represents one of the focal points toward the solution of the cosmological Lithium abundance problem, and whose only measurement, at thermal energy, dates back to 1963. The apparently unsurmountable experimental difficulties stemming from the huge {sup 7}Be γ-activity, along with the lack of a suitable neutron beam facility, had so far prevented further measurements. The detection system is subject to considerable radiation damage, but is capable of disentangling the rare reaction signals from the very high background. This newly developed setup could likely be useful also to study other challenging reactions requiring the detectors to be installed directly in the neutron beam.

  5. Moderator materials for the Spallation Neutron Source

    International Nuclear Information System (INIS)

    Charlton, L.A.

    1999-01-01

    The Spallation Neutron Source (SNS) is a neutron source providing intense neutron fluxes that will be used for performing a large variety of neutron scattering experiments. SNS is to be completed and start operation in 2005. Protons will be accelerated to 1 GeV, stored in an accumulator ring, and then injected into a neutron-producing target. After leaving the target (Hg in the ca/se of SNS), the neutrons are prepared for experiments by first using a moderator to impose energy and width requirements on the neutron pulse. One of the most important ingredients is the moderator material. Four materials that are commonly used and that were considered for use in SNS are liquid hydrogen (L-H 2 ), liquid water (L-H 2 O), liquid methane (L-CH 4 ), and solid methane (S-CH 4 ). The spectra (neutron current versus neutron energy) for these four materials are shown. As may be seen, at low neutron energies ( 4 , which produces up to four times as many neutrons in this energy range as L-H 2 . The problem with the material is the internal storage of energy that can be spontaneously and explosively released. At energies of just above 10 MeV, the most effective moderator material is L-CH 4 . Polymerization problems, however, preclude its use at high powers (again such as in SNS), where the buildup of undesirable materials becomes prohibitive. This is, however, an important energy range for neutron experiments. Preliminary consideration is being given to a composite moderator that contains two adjacent sections, one of L-H 2 and one of L-H 2 O, which produces a spectrum that is very similar to L-CH 4

  6. Emission of high-energy charged particles at 00 in Ne-induced reactions

    International Nuclear Information System (INIS)

    Borcea, C.; Gierlik, E.; Kalinin, A.M.; Kalpakchieva, R.; Oganessia, Yu.Ts.; Pawlat, T.; Penionzhkevich, Yu.E.; Ryakhlyuk, A.V.

    1982-01-01

    Inclusive energy spectra have been measured for light charged particles emitted in the bombardment of 232 Th, 181 Ta, sup(nat)Ti and 12 C targets by 22 Ne ions at 178 MeV and sup(nat)Ti target by 20 Ne ions at 196 MeV. The reaction products were analysed and detected by means of a ΔE-E telescope placed in the focal plane of a magnetic spectrometer located at an angle of 0 deg with respect to the beam direction. In all the reactions studied light charged particles with an energy close to the respective calculated kinematic limit for a two-body exit channel are produced with relatively great probability. The results obtained make it possible to draw some conclusions about the reaction mechanism involving the emission of light charged particles

  7. Energy gains from lattice-enabled nuclear reactions

    International Nuclear Information System (INIS)

    Nagel, David J.

    2015-01-01

    The energy gain of a system is defined as the ratio of its output energy divided by the energy provided to operate the system. Most familiar systems have energy gains less than one due to various inefficiencies. By contrast, lattice-enabled nuclear reactions (LENR) offer high energy gains. Theoretical values in excess of 1000 are possible. Energy gains over 100 have already been reported. But, they have not yet been sustained for commercially significant durations. This article summarizes the current status of LENR energy gains. (author)

  8. Energy and Molecules from Photochemical/Photocatalytic Reactions. An Overview

    Directory of Open Access Journals (Sweden)

    Davide Ravelli

    2015-01-01

    Full Text Available Photocatalytic reactions have been defined as those processes that require both a (not consumed catalyst and light. A previous definition was whether such reactions brought a system towards or away from the (thermal equilibrium. This consideration brings in the question whether a part of the photon energy is incorporated into the photochemical reaction products. Data are provided for representative organic reactions involving or not molecular catalysts and show that energy storage occurs only when a heavily strained structure is generated, and in that case only a minor part of photon energy is actually stored (ΔG up to 25 kcal·mol−1. The green role of photochemistry/photocatalysis is rather that of forming highly reactive intermediates under mild conditions.

  9. MEGAPIE, a 1 MW pilot experiment for a liquid metal spallation target

    Energy Technology Data Exchange (ETDEWEB)

    Bauer, G.S. [Paul Scherrer Institut, Spallation Neutron Source Division, Villigen-PSI (Switzerland); Salvatores, M. [CEA Cadarache, Direction des Reacteurs Nucleaires, Saint-Paul-lez-Durance Cedex (France); Heusener, G. [Forschungszentrum Karlsruhe, Projekt Nukleare Sicherheitsforschung, Karlsruhe (Germany)

    2001-03-01

    MEGAPIE (Megawatt Pilot Target Experiment) is an initiative launched by Commissariat a l'Energie Atomique, Cadarache (France) and Forschungszentrum Karlsruhe (Germany) in collaboration with Paul Scherrer Institut (Switzerland), to demonstrate, in an international collaboration, the feasibility of a liquid lead bismuth target for spallation facilities at a beam power level of 1 MW. Such a target is under consideration for various concepts of accelerator driven systems (ADS) to be used in transmutation of nuclear waste and other applications world-wide. It also has the potential of increasing significantly the thermal neutron flux available at the spallation neutron source (SINQ) for neutron scattering. SINQ's beam power being close to 1 MW already, this facility offers a unique opportunity to realize such an experiment with a reasonably small number of new ancillary systems. The paper describes the basic features of the experiment and its boundary conditions, the technical concept of the target and underlying research carried out at participating laboratories. (author)

  10. MEGAPIE, a 1 MW pilot experiment for a liquid metal spallation target

    International Nuclear Information System (INIS)

    Bauer, G.S.; Salvatores, M.; Heusener, G.

    2001-01-01

    MEGAPIE (Megawatt Pilot Target Experiment) is an initiative launched by Commissariat a l'Energie Atomique, Cadarache (France) and Forschungszentrum Karlsruhe (Germany) in collaboration with Paul Scherrer Institut (Switzerland), to demonstrate, in an international collaboration, the feasibility of a liquid lead bismuth target for spallation facilities at a beam power level of 1 MW. Such a target is under consideration for various concepts of accelerator driven systems (ADS) to be used in transmutation of nuclear waste and other applications world-wide. It also has the potential of increasing significantly the thermal neutron flux available at the spallation neutron source (SINQ) for neutron scattering. SINQ's beam power being close to 1 MW already, this facility offers a unique opportunity to realize such an experiment with a reasonably small number of new ancillary systems. The paper describes the basic features of the experiment and its boundary conditions, the technical concept of the target and underlying research carried out at participating laboratories. (author)

  11. On the geometric nature of high energy nucleus-nucleus reaction cross sections

    International Nuclear Information System (INIS)

    Townsend, L.W.; Wilson, J.W.; Bidasaria, H.B.

    1982-01-01

    Within the context of a high energy double-folding optical potential approximation to the exact nucleus-nucleus multiple-scattering series, eikonal scattering theory is used to investigate the validity of geometric reaction cross sections in relativistic heavy ion collisions. The potential used includes a finite range interaction and nuclear single-particle densities extracted from nuclear charge distributions by unfolding the proton charge distribution. Pauli correlation effects are also included in an approximate way. The sensitivity of the predictions to be assumed interaction, Pauli correlation approximation, and nuclear density distributions is investigated. These results are in agreement with early predictions concerning the geometric nature of relativistic heavy ion collisions and in disagreement with a recent analysis, utilizing the zero range approximation, which suggested otherwise. Reasons for the lack of agreement between the analyses are also presented. Finally, approximate applicability for geometric reaction cross sections are determined

  12. The very low angle detector for high-energy inelastic neutron scattering on the VESUVIO spectrometer

    Energy Technology Data Exchange (ETDEWEB)

    Perelli Cippo, E.; Gorini, G.; Tardocchi, M. [Dipartimento di Fisica ' G. Occhialini' , Universita degli Studi di Milano-Bicocca, Piazza della Scienza 3, 20126 Milano (Italy); Pietropaolo, A. [Dipartimento di Fisica ' G. Occhialini' , CNISM-Universita degli Studi di Milano-Bicocca, Piazza della Scienza 3, 20126 Milano (Italy); NAST Center - Nanoscienze-Nanotecnologie-Strumentazione, Universita degli Studi di Roma Tor Vergata, via della Ricerca Scientifica 1, 00133 Roma (Italy)], E-mail: antonino.pietropaolo@mib.infn.it; Andreani, C.; Senesi, R. [Dipartimento di Fisica and Centro NAST - Nanoscienze-Nanotecnologie-Strumentazione, Universita degli Studi di Roma Tor Vergata, via della Ricerca Scientifica 1, 00133 Roma (Italy); Rhodes, N.J.; Schooneveld, E.M. [ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire 0QX OX11 (United Kingdom)

    2008-05-01

    The Very Low Angle Detector (VLAD) bank has been installed on the VESUVIO spectrometer at the ISIS spallation neutron source. The new device allows for high-energy inelastic neutron scattering measurements, at energies above 1 eV, maintaining the wave vector transfer lower than 10A{sup -1}. This opens a still unexplored region of the kinematical (q,{omega}) space, enabling new and challenging experimental investigations in condensed matter. This paper describes the main instrumental features of the VLAD device, including instrument design, detector response, and calibration procedure.

  13. High-lying neutron hole strengths observed in pick-up reactions

    International Nuclear Information System (INIS)

    Gales, S.

    1980-01-01

    Neutron-hole states in orbits well below the Fermi surface have been observed in a number of medium-heavy nuclei from A=90 to 209 using one nucleon pick-up reactions. The excitation energies, angular distributions of such broad and enhanced structures will be discussed. The fragmentation of the neutron-hole strengths as well as the spreading of such simple mode of excitations into more complex states are compared to recent calculations within the quasiparticle-phonon or the single particle-vibration coupling nuclear models. We report on recent measurements of J for inner-hole states in 89 Zr and 115 Sn 119 Sn using the analyzing power of the (p,d) and (d,t) reactions. Large enhancement of cross-sections are observed at high excitation energy in the study of the (p,t) reactions on Zr, Cd, Sn, Te and Sm isotopes. The systematic features of such high-lying excitation are related to the ones observed in one neutron pick-up experiments. The origin of such concentration of two neutron-hole strengths in Cd and Sn isotopes will be discussed. Preliminary results obtained in the study of the (α, 6 He) reaction at 218 MeV incident energy on 90 Zr, 118 Sn and 208 Pb targets are presented and compared to the (p,t) results. Finally the properties of hole-analog states populated in neutron pick-up reactions (from 90 Zr to 208 Pb) will be presented

  14. Nuclear reaction models - source term estimation for safety design in accelerators

    International Nuclear Information System (INIS)

    Nandy, Maitreyee

    2013-01-01

    Accelerator driven subcritical system (ADSS) employs proton induced spallation reaction at a few GeV. Safety design of these systems involves source term estimation in two steps - multiple fragmentation of the target and n+γ emission through a fast process followed by statistical decay of the primary fragments. The prompt radiation field is estimated in the framework of quantum molecular dynamics (QMD) theory, intra-nuclear cascade or Monte Carlo calculations. A few nuclear reaction model codes used for this purpose are QMD, JQMD, Bertini, INCL4, PHITS, followed by statistical decay codes like ABLA, GEM, GEMINI, etc. In the case of electron accelerators photons and photoneutrons dominate the prompt radiation field. High energy photon yield through Bremsstrahlung is estimated in the framework of Born approximation while photoneutron production is calculated using giant dipole resonance and quasi-deuteron formation cross section. In this talk hybrid and exciton PEQ models and QMD formalism will be discussed briefly

  15. Resolution of the VESUVIO spectrometer for High-energy Inelastic Neutron Scattering experiments

    International Nuclear Information System (INIS)

    Imberti, S.; Andreani, C.; Garbuio, V.; Gorini, G.; Pietropaolo, A.; Senesi, R.; Tardocchi, M.

    2005-01-01

    New perspectives for epithermal neutron spectroscopy have been opened up as a result of the development of the Resonance Detector and its use on inverse geometry time-of-flight spectrometers at spallation sources. A special application of the Resonance Detector is the Very Low Angle Detector Bank (VLAD) for the VESUVIO spectrometer at ISIS, operating in the angular range 1 deg. -1 ) and high energy (unlimited) transfer -bar ω>500meV, a regime so far inaccessible to experimental studies on condensed matter systems. The HINS measurements complement the Deep Inelastic Neutron Scattering (DINS) measurements performed on VESUVIO in the high wavevector q(20A -1 -1 ) and high energy transfer (-bar ω>1eV), where the short-time single-particle dynamics can be sampled. This paper will revise the main components of the resolution for HINS measurements of VESUVIO. Instrument performances and examples of applications for neutron scattering processes at high energy and at low wavevector transfer are discussed

  16. Intermediate- and high-energy reactions of uranium with neon and carbon

    International Nuclear Information System (INIS)

    McGaughey, P.L.

    1982-11-01

    Target fragment production from the interactions of 1.0, 3.0, 4.8, and 12 GeV 12 C and 5.0, 8.0, 20, and 42 GeV 20 Ne with uranium has been measured using off-line gamma-ray spectroscopic techniques. The experimental charge and mass yield distributions are generally consistent with the concepts of limiting fragmentation and factorization at energies of 3.0 GeV and above. The total projectile kinetic energy was found to be the relevant scaling parameter for the comparison of reactions induced by projectiles of different sizes. Light fragments with mass number less than 60 were found to violate limiting fragmentation, and had excitation functions that were strongly increasing with projectile energy until 8.0 to 12.0 GeV. With the 1.0 GeV 12 C beam the pattern of mass yields was quite different from that of all the other reactions, with the normal peak in the fission mass region (80 < A < 145), but with much lower yields below mass number 60 and between mass numbers 145 and 210, indicating that these fragments are formed primarily in very energetic reactions in which large excitation energies are transferred to and significant amounts of mass are removed from the target nucleus. Theoretical predictions of the intra-nuclear cascade, nuclear fireball, and nuclear firestreak models are compared with the experimental results. The intra-nuclear cascade and nuclear firestreak models are both able to predict the general shapes of the experimental distributions, with the exception of the yields for the lightest fragments

  17. Behavior of structural and target materials irradiated in spallation neutron environments

    Energy Technology Data Exchange (ETDEWEB)

    Stubbins, J.F. [Univ. of Illinois, Urbana, IL (United States); Wechsler, M. [North Carolina State Univ., Raleigh, NC (United States); Borden, M. [Los Alamos National Laboratory, NM (United States)] [and others

    1995-10-01

    This paper describes considerations for selection of structural and target materials for accelerator-driven neutron sources. Due to the operating constraints of proposed accelerator-driven neutron sources, the criteria for selection are different than those commonly applied to fission and fusion systems. Established irradiation performance of various alloy systems is taken into account in the selection criteria. Nevertheless, only limited materials performance data are available which specifically related to neutron energy spectra anticipated for spallation sources.

  18. Behavior of structural and target materials irradiated in spallation neutron environments

    International Nuclear Information System (INIS)

    Stubbins, J.F.; Wechsler, M.; Borden, M.

    1995-01-01

    This paper describes considerations for selection of structural and target materials for accelerator-driven neutron sources. Due to the operating constraints of proposed accelerator-driven neutron sources, the criteria for selection are different than those commonly applied to fission and fusion systems. Established irradiation performance of various alloy systems is taken into account in the selection criteria. Nevertheless, only limited materials performance data are available which specifically related to neutron energy spectra anticipated for spallation sources

  19. Extended sudden approximation model for high-energy nucleon removal reactions

    Energy Technology Data Exchange (ETDEWEB)

    Carstoiu, F.; Sauvan, E.; Orr, N.A. [Caen Univ., Lab. de Physique Corpusculaire, Institut des Sciences de la Matiere et du Rayonnement, IN2P3-CNRS ISMRA, 14 (France); Carstoiu, F. [IFIN-HH, Bucharest-Magurele (Romania); Bonaccorso, A. [Istituto Nazionale di Fisica Nucleare, Pisa (Italy)

    2004-04-01

    A model based on the sudden approximation has been developed to describe high energy single nucleon removal reactions. Within this approach, which takes as its starting point the formalism of Hansen, the nucleon-removal cross section and the full 3-dimensional momentum distributions of the core fragments including absorption, diffraction, Coulomb and nuclear-Coulomb interference amplitudes, have been calculated. The Coulomb breakup has been treated to all orders for the dipole interaction. The model has been compared to experimental data for a range of light, neutron-rich psd-shell nuclei. Good agreement was found for both the inclusive cross sections and momentum distributions. In the case of {sup 17}C, comparison is also made with the results of calculations using the transfer-to-the-continuum model. The calculated 3-dimensional momentum distributions exhibit longitudinal and transverse momentum components that are strongly coupled by the reaction for s-wave states, whilst no such effect is apparent for d-waves. Incomplete detection of transverse momenta arising from limited experimental acceptances thus leads to a narrowing of the longitudinal distributions for nuclei with significant s-wave valence neutron configurations, as confirmed by the data. Asymmetries in the longitudinal momentum distributions attributed to diffractive dissociation are also explored. (authors)

  20. Extended sudden approximation model for high-energy nucleon removal reactions

    International Nuclear Information System (INIS)

    Carstoiu, F.; Sauvan, E.; Orr, N.A.; Carstoiu, F.; Bonaccorso, A.

    2004-04-01

    A model based on the sudden approximation has been developed to describe high energy single nucleon removal reactions. Within this approach, which takes as its starting point the formalism of Hansen, the nucleon-removal cross section and the full 3-dimensional momentum distributions of the core fragments including absorption, diffraction, Coulomb and nuclear-Coulomb interference amplitudes, have been calculated. The Coulomb breakup has been treated to all orders for the dipole interaction. The model has been compared to experimental data for a range of light, neutron-rich psd-shell nuclei. Good agreement was found for both the inclusive cross sections and momentum distributions. In the case of 17 C, comparison is also made with the results of calculations using the transfer-to-the-continuum model. The calculated 3-dimensional momentum distributions exhibit longitudinal and transverse momentum components that are strongly coupled by the reaction for s-wave states, whilst no such effect is apparent for d-waves. Incomplete detection of transverse momenta arising from limited experimental acceptances thus leads to a narrowing of the longitudinal distributions for nuclei with significant s-wave valence neutron configurations, as confirmed by the data. Asymmetries in the longitudinal momentum distributions attributed to diffractive dissociation are also explored. (authors)

  1. Tensile mechanical properties of a stainless steel irradiated up to 19 dpa in the Swiss spallation neutron source

    Energy Technology Data Exchange (ETDEWEB)

    Saito, Shigeru, E-mail: saito.shigeru@jaea.go.jp [JAEA, J-PARC Center, Tokai-mura, Ibaraki-ken 319-1195 (Japan); Kikuchi, Kenji [Ibaraki Univ., iFRC, Tokai-mura, Ibaraki-ken 319-1106 (Japan); Hamaguchi, Dai [JAEA, J-PARC Center, Tokai-mura, Ibaraki-ken 319-1195 (Japan); Usami, Kouji; Endo, Shinya; Ono, Katsuto; Matsui, Hiroki [JAEA, Dept. of Hot Laboratories, Tokai-mura, Ibaraki-ken 319-1195 (Japan); Kawai, Masayoshi [KEK, Tsukuba-shi, Ibaraki-ken 305-0801 (Japan); Dai, Yong [PSI, Spallation Source Division, Villigen PSI (Switzerland)

    2012-12-15

    To evaluate the lifetime of the beam window of an accelerator-driven transmutation system (ADS), post irradiation examination (PIE) of the STIP (SINQ target irradiation program, SINQ; Swiss spallation neutron source) specimens was carried out. The specimens tested in this study were made from the austenitic steel Japan primary candidate alloy (JPCA). The specimens were irradiated at SINQ Target 4 (STIP-II) with high-energy protons and spallation neutrons. The irradiation conditions were as follows: the proton energy was 580 MeV, irradiation temperatures ranged from 100 to 430 Degree-Sign C, and displacement damage levels ranged from 7.1 to 19.5 dpa. Tensile tests were performed in air at room temperature (RT), 250 Degree-Sign C and 350 Degree-Sign C. Fracture surface observation after the tests was done by Scanning electron microscope (SEM). Results of the tensile tests performed at R.T. showed the extra hardening of JPCA at higher dose compared to the fission neutron irradiated data. At the higher temperatures, 250 Degree-Sign C and 350 Degree-Sign C, the extra hardening was not observed. Degradation of ductility bottomed around 10 dpa, and specimens kept their ductility until 19.5 dpa. All specimens fractured in ductile manner.

  2. High energy halogen atom reactions activated by nuclear transformations. Progress report, February 15-December 31, 1984

    International Nuclear Information System (INIS)

    1985-01-01

    Energetic halogen atoms or ions, activated by various nuclear transformations are studied in gas, high pressure and condensed phase saturated and unsaturated hydrocarbons, halomethanes, and liquid and solid aqueous solutions of biomolecular and organic solutes in order to understand better the mechanisms and dynamics of high energy monovalent species. The experimental program and its goals remain the same, consisting of four interrelated areas: (1) The stereochemistry of energetic 18 F, /sup 34m/Cl, and 38 Cl substitution reactions with chiral molecules in the gas and condensed phase is studied. (2) The gas to condensed state transition in halogen high energy chemistry, involving energetic chlorine, bromine, and iodine reactions in halomethanes, saturated and unsaturated hydrocarbons and aqueous solutions of biomolecules and alkyl halides is being investigated in more detail. Current attention is given to defining the nature of the enhancement yields in the condensed phase. Specifically, energetic halogen reactions in liquid and frozen aqueous solutions or organic and biomolecular solutes are studied. (3) Reactions of bromine and iodine activated by isomeric transition with halogenated biomolecular and organic solutes in liquid and frozen aqueous solutions are being studied in an attempt to learn more about the activation events in the condensed phase. (4) The applications of hot chemistry techniques and theory to neutron activation analysis of biological systems are being continued. Current attention is given to developing procedures for trace molecular determinations in biological systems. The applications of hot halogen atoms as site indicators in liquid and frozen aqueous solutions of halogenated bases and nucleosides are currently being developed. 14 references

  3. Characterization of the radiation background at the Spallation Neutron Source

    International Nuclear Information System (INIS)

    DiJulio, Douglas D.; Cherkashyna, Nataliia; Scherzinger, Julius; Khaplanov, Anton; Pfeiffer, Dorothea; Cooper-Jensen, Carsten P.; Fissum, Kevin G.; Kanaki, Kalliopi; Kirstein, Oliver; Hall-Wilton, Richard J.; Bentley, Phillip M.; Ehlers, Georg; Gallmeier, Franz X.; Hornbach, Donald E.; Iverson, Erik B.; Newby, Robert J.

    2016-01-01

    We present a survey of the radiation background at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory, TN, USA during routine daily operation. A broad range of detectors was used to characterize primarily the neutron and photon fields throughout the facility. These include a WENDI-2 extended range dosimeter, a thermoscientific NRD, an Arktis 4 He detector, and a standard NaI photon detector. The information gathered from the detectors was used to map out the neutron dose rates throughout the facility and also the neutron dose rate and flux profiles of several different beamlines. The survey provides detailed information useful for developing future shielding concepts at spallation neutron sources, such as the European Spallation Source (ESS), currently under construction in Lund, Sweden. (paper)

  4. Light nuclides produced in the proton-induced spallation of {sup 238}U at 1 GeV

    Energy Technology Data Exchange (ETDEWEB)

    Ricciardi, M.V.; Armbruster, P. [Gesellschaft fuer Schwerionenforschung mbH, Darmstadt (Germany); Benlliure, J. [Universidad de Santiago de Compostela (ES)] [and others

    2005-09-01

    The production of light and intermediate-mass nuclides formed in the reaction {sup 1}H+{sup 238}U at 1 GeV was measured at the fragment separator (FRS) at GSI, Darmstadt. The experiment was performed in inverse kinematics, shooting a 1 A GeV {sup 238}U beam on a thin liquid-hydrogen target. 254 isotopes of all elements in the range 7{<=}Z{<=}37 were unambiguously identified, and the velocity distributions of the produced nuclides were determined with high precision. The results show that the nuclides are produced in a very asymmetric binary decay of heavy nuclei originating from the spallation of uranium. All the features of the produced nuclides merge with the characteristics of the fission products as their mass increases. (orig.)

  5. Safety analysis and lay-out aspects of shieldings against particle radiation at the example of spallation facilities in the megawatt range; Sicherheitstechnische Analyse und Auslegungsaspekte von Abschirmungen gegen Teilchenstrahlung am Beispiel von Spallationsanlagen im Megawatt Bereich

    Energy Technology Data Exchange (ETDEWEB)

    Hanslik, R.

    2006-08-15

    This paper discusses the shielding of particle radiation from high current accelerators, spallation neutron sources and so called ADS-facilities (Accelerator Driven Systems). ADS-facilities are expected to gain importance in the future for transmutation of long-lived isotopes from fission reactors as well as for energy production. In this paper physical properties of the radiation as well as safety relevant requirements and corresponding shielding concepts are discussed. New concepts for the layout and design of such shielding are presented. Focal point of this work will be the fundamental difference between conventional fission reactor shielding and the safety relevant issues of shielding from high-energy radiation. Key point of this paper is the safety assessment of shielding issues of high current accelerators, spallation targets and ADS-blanket systems as well as neutron scattering instruments at spallation neutron sources. Safety relevant shielding requirements are presented and discussed. For the layout and design of the shielding for spallation sources computer base calculations methods are used. A discussion and comparison of the most important methods like semi-empirical, deterministic and stochastic codes are presented. Another key point within the presented paper is the discussion of shielding materials and their shielding efficiency concerning different types of radiation. The use of recycling material, as a cost efficient solution, is discussed. Based on the conducted analysis, flowcharts for a systematic layout and design of adequate shielding for targets and accelerators have been developed and are discussed in this paper. By use of these flowcharts layout and engineering design of future ADS-facilities can be performed. (orig.)

  6. Synchrotron based spallation neutron source concepts

    International Nuclear Information System (INIS)

    Cho, Y.

    1998-01-01

    During the past 20 years, rapid-cycling synchrotrons (RCS) have been used very productively to generate short-pulse thermal neutron beams for neutron scattering research by materials science communities in Japan (KENS), the UK (ISIS) and the US (IPNS). The most powerful source in existence, ISIS in the UK, delivers a 160-kW proton beam to a neutron-generating target. Several recently proposed facilities require proton beams in the MW range to produce intense short-pulse neutron beams. In some proposals, a linear accelerator provides the beam power and an accumulator ring compresses the pulse length to the required ∼ 1 micros. In others, RCS technology provides the bulk of the beam power and compresses the pulse length. Some synchrotron-based proposals achieve the desired beam power by combining two or more synchrotrons of the same energy, and others propose a combination of lower and higher energy synchrotrons. This paper presents the rationale for using RCS technology, and a discussion of the advantages and disadvantages of synchrotron-based spallation sources

  7. High energy magnetic excitations

    International Nuclear Information System (INIS)

    Endoh, Yasuo

    1988-01-01

    The report emphasizes that the current development in condensed matter physics opens a research field fit to inelastic neutron scattering experiments in the eV range which is easilly accessed by spallation neutron sources. Several important subjects adopted at thermal reactors are shown. It is desired to extend the implementation of the spectroscopic experiments for investigation of higher energy magnetic excitations. For La 2 CuO 4 , which is the mother crystal of the first high Tc materials found by Bednortz and Muller, it seems to be believed that the magnetism is well characterized by the two-dimensional Heisenberg antiferromagnetic Hamiltonian, and it is widely accepted that the magnetism is a most probable progenitor of high Tc superconductors. The unusual properties of spin correlations in this crystal have been studied extensively by standard neutron scattering techniques with steady neutrons at BNL. FeSi is not ordered magnetically but shows a very unique feature of temperature induced magnetism, which also has been studied extensively by using the thermal neutron scattering technique at BNL. In these experiments, polarized neutrons are indispensable to extract the clean magnetic components out of other components of non-magnetic scattering. (N.K.)

  8. CFD analysis of the HYPER spallation target

    International Nuclear Information System (INIS)

    Cho, Chungho; Tak, Nam-il; Choi, Jae-Hyuk; Lee, Yong-Bum

    2008-01-01

    KAERI (Korea Atomic Energy Research Institute) is developing an accelerator driven system (ADS) named HYPER (HYbrid Power Extraction Reactor) for a transmutation of long-lived nuclear wastes. One of the challenging tasks for the HYPER system is to design a large spallation target with a beam power of 15-25 MW. The paper focuses on a thermal-hydraulic analysis of the active part of the HYPER target. Computational fluid dynamics (CFD) analysis was performed by using a commercial code CFX 5.7.1. Several advanced turbulence models with different grid structures were applied. The CFX results reveal a significant impact of the turbulence model on the window temperature. Particularly, the k-ε model predicts the lowest window temperature among the five investigated turbulence models

  9. Fundamental neutron physics at a 1 MW long pulse spallation neutron source

    International Nuclear Information System (INIS)

    Greene, G.L.

    1995-01-01

    Modern neutron sources and modern neutron science share a common origin in mid twentieth century scientific investigations concerned with the study of the fundamental interactions between elementary particles. Since the time of that common origin, neutron science and the study of elementary particles have evolved into quite disparate disciplines. The neutron became recognized as a powerful tool for the study of condensed matter with modern neutron sources being primarily used (and primarily justified) as tools for condensed matter research. The study of elementary particles has, of course, led to the development of rather different tools and is now dominated by activities carried out at extremely high energies. Notwithstanding this trend, the study of fundamental interactions using neutrons has continued and remains a vigorous activity at many contemporary neutron sources. This research, like neutron scattering research, has benefited enormously by the development of modern high flux neutron facilities. Future sources, particularly high power spallation sources, offer exciting possibilities for the continuation of this program of research

  10. Differential cross section measurements for the 6Li(n,t)alpha reaction in the few MeV region

    Energy Technology Data Exchange (ETDEWEB)

    Devlin, Matthew J [Los Alamos National Laboratory; Taddeucci, Terence N [Los Alamos National Laboratory; Hale, Gerald M [Los Alamos National Laboratory; Haight, Robert C [Los Alamos National Laboratory; O' Donnell, Johhn M [Los Alamos National Laboratory

    2008-01-01

    New measured differential cross sections of tritons and alpha particles following the {sup 6}Li(n,t){alpha} reaction are reported for incident neutron energies between 0.2 and approximately 20 MeV. The neutrons were produced by spallation at the WNR facility at the Los Alamos Neutron Science CEnter (LANSCE), with the incident neutron energy determined by the time-of-flight method. Four E-{Delta}E telescopes were used at eight laboratory angles. These data have been incorporated into a prior R-matrix fit for the compound {sup 7}Li system, and result in an (n,t) reaction cross section that is 4% to 10% higher than previous evaluations in the 1-3 MeV incident neutron energy region.

  11. Exploring nuclear reactions relevant to Stellar and Big-Bang Nucleosynthesis using High-Energy-Density plasmas at OMEGA and the NIF

    Science.gov (United States)

    Gatu Johnson, M.

    2017-10-01

    Thermonuclear reaction rates and nuclear processes have been explored traditionally by means of accelerator experiments, which are difficult to execute at conditions relevant to Stellar Nucleosynthesis (SN) and Big Bang Nucleosynthesis (BBN). High-Energy-Density (HED) plasmas closely mimic astrophysical environments and are an excellent complement to accelerator experiments in exploring SN and BBN-relevant nuclear reactions. To date, our work using HED plasmas at OMEGA and NIF has focused on the complementary 3He+3He, T+3He and T +T reactions. First studies of the T +T reaction indicated the significance of the 5He ground-state resonance in the T +T neutron spectrum. Subsequent T +T experiments showed that the strength of this resonance varies with center-of-mass (c-m) energy in the range of 16-50 keV, a variation that is not fundamentally understood. Studies of the 3He+3He and T+3He reactions have also been conducted at OMEGA at c-m energies of 165 keV and 80 keV, respectively, and the results revealed three things. First, a large cross section for the T+3He- γ branch can be ruled out as an explanation for the anomalously high abundance of 6Li in primordial material. Second, the results contrasted to theoretical modeling indicate that the mirror-symmetry assumption is not enough to capture the differences between T +T and 3He+3He reactions. Third, the elliptical spectrum assumed in the analysis of 3He+3He data obtained in accelerator experiments is incorrect. Preliminary data from recent experiments at the NIF exploring the 3He+3He reaction at c-m energies of 60 keV and 100 keV also indicate that the underlying physics changes with c-m energy. In this talk, we describe these findings and future directions for exploring light-ion reactions at OMEGA and the NIF. The work was supported in part by the US DOE, LLE, and LLNL.

  12. A fission ionization detector for neutron flux measurements at a spallation source

    Energy Technology Data Exchange (ETDEWEB)

    Wender, S.A. (Los Alamos National Lab., Los Alamos, NM (United States)); Balestrini, S. (Los Alamos National Lab., Los Alamos, NM (United States)); Brown, A. (Los Alamos National Lab., Los Alamos, NM (United States)); Haight, R.C. (Los Alamos National Lab., Los Alamos, NM (United States)); Laymon, C.M. (Los Alamos National Lab., Los Alamos, NM (United States)); Lee, T.M. (Los Alamos National Lab., Los Alamos, NM (United States)); Lisowski, P.W. (Los Alamos National Lab., Los Alamos, NM (United States)); McCorkle, W. (Los Alamos National Lab., Los Alamos, NM (United States)); Nelson, R.O. (Los Alamos National Lab., Los Alamos, NM (United States)); Parker, W. (Los Alamos National Lab., Los Alamos, NM (United States)); Hill, N.W. (Oak Ridge National Lab., Oak Ridge, TN (United States))

    1993-11-15

    The construction of a neutron flux monitor that can measure absolute neutron intensities in the neutron energy range from below 1 MeV to over 500 MeV is described. The detector consists of an ionization chamber with several thin deposits of fissionable material. The ionization chamber is thin enough that it does not significantly affect the neutron beam and may be left in the neutron flight path during experimental measurements to continuously monitor the beam flux. The use of this monitor at the continuous-energy spallation neutron source at the WNR target area at LAMPF is described. (orig.)

  13. A fission ionization detector for neutron flux measurements at a spallation source

    International Nuclear Information System (INIS)

    Wender, S.A.; Balestrini, S.; Brown, A.; Haight, R.C.; Laymon, C.M.; Lee, T.M.; Lisowski, P.W.; McCorkle, W.; Nelson, R.O.; Parker, W.; Hill, N.W.

    1993-01-01

    The construction of a neutron flux monitor that can measure absolute neutron intensities in the neutron energy range from below 1 MeV to over 500 MeV is described. The detector consists of an ionization chamber with several thin deposits of fissionable material. The ionization chamber is thin enough that it does not significantly affect the neutron beam and may be left in the neutron flight path during experimental measurements to continuously monitor the beam flux. The use of this monitor at the continuous-energy spallation neutron source at the WNR target area at LAMPF is described. (orig.)

  14. Radioactive nuclide production and isomeric state branching ratios in P + W reactions to 200 mev

    International Nuclear Information System (INIS)

    Young, P.G.; Chadwick, M.B.

    1995-01-01

    Calculations of nuclide yields from spallation reactions usually assume that the products are formed in their ground states. We are performing calculations of product yields from proton reactions on tungsten isotopes that explicitly account for formation of the residual nuclei in excited states. The Hauser-Feshbach statistical/preequilibrium code GNASH, with full accounting for angular momentum conservation and electromagnetic transitions, is utilized in the calculations. We present preliminary results for isomer branching ratios for proton reactions to 200 MeV for several products including the 31-y, 16+ state in l78 Hf and the 25-d, 25/2- state in 179 Hf. Knowledge of such branching ratios, might be important for concepts such as accelerator production of tritium that utilize intermediate-energy proton reactions on tungsten

  15. Reaction mechanism and reaction coordinates from the viewpoint of energy flow

    Energy Technology Data Exchange (ETDEWEB)

    Li, Wenjin; Ma, Ao, E-mail: aoma@uic.edu [Department of Bioengineering, The University of Illinois at Chicago, 851 South Morgan Street, Chicago, Illinois 60607 (United States)

    2016-03-21

    Reaction coordinates are of central importance for correct understanding of reaction dynamics in complex systems, but their counter-intuitive nature made it a daunting challenge to identify them. Starting from an energetic view of a reaction process as stochastic energy flows biased towards preferred channels, which we deemed the reaction coordinates, we developed a rigorous scheme for decomposing energy changes of a system, both potential and kinetic, into pairwise components. The pairwise energy flows between different coordinates provide a concrete statistical mechanical language for depicting reaction mechanisms. Application of this scheme to the C{sub 7eq} → C{sub 7ax} transition of the alanine dipeptide in vacuum revealed novel and intriguing mechanisms that eluded previous investigations of this well studied prototype system for biomolecular conformational dynamics. Using a cost function developed from the energy decomposition components by proper averaging over the transition path ensemble, we were able to identify signatures of the reaction coordinates of this system without requiring any input from human intuition.

  16. Reaction mechanism and reaction coordinates from the viewpoint of energy flow

    International Nuclear Information System (INIS)

    Li, Wenjin; Ma, Ao

    2016-01-01

    Reaction coordinates are of central importance for correct understanding of reaction dynamics in complex systems, but their counter-intuitive nature made it a daunting challenge to identify them. Starting from an energetic view of a reaction process as stochastic energy flows biased towards preferred channels, which we deemed the reaction coordinates, we developed a rigorous scheme for decomposing energy changes of a system, both potential and kinetic, into pairwise components. The pairwise energy flows between different coordinates provide a concrete statistical mechanical language for depicting reaction mechanisms. Application of this scheme to the C 7eq → C 7ax transition of the alanine dipeptide in vacuum revealed novel and intriguing mechanisms that eluded previous investigations of this well studied prototype system for biomolecular conformational dynamics. Using a cost function developed from the energy decomposition components by proper averaging over the transition path ensemble, we were able to identify signatures of the reaction coordinates of this system without requiring any input from human intuition.

  17. Proceedings of the third specialists` meeting on high energy nuclear data

    Energy Technology Data Exchange (ETDEWEB)

    Fukahori, Tokio [ed.

    1998-11-01

    This report is the Proceedings of the Third Specialists` Meeting on High Energy Nuclear Data. The meeting was held on March 30-31, 1998, at the Tokai Research Establishment of Japan Atomic Energy Research Institute with the participation of forty-odd specialists, who were the evaluators, theorists, experimentalists and users of high energy nuclear data including the members of the Japanese Nuclear Data Committee. The need of the high energy nuclear data up to a few Gev has been stressed in the meeting for many applications, such as spallation neutron sources for radioactive waste treatment, accelerator shielding design, medical isotope production, radiation therapy, the effects of space radiation on astronauts and their equipments, and the cosmic history of meteorites and other galactic substances. Since the Second Specialists` Meeting in 1995, such an evaluation activity in Japan has been grown and the results are accumulated. Foreign activities of high energy nuclear data evaluation are also being increased. According to the above situation, with the view point of reviewing and validating an evaluated high energy nuclear data file, project of high energy nuclear data file production, differential and integral experiments, status of evaluation and reviewing methods, processing and transport calculation methods, benchmark tests, international trends, etc. were discussed. The 16 of the presented papers are indexed individually. (J.P.N.)

  18. A long-wavelength target station for the spallation neutron source

    International Nuclear Information System (INIS)

    Carpenter, J.M.; Mason, T.E.

    2005-01-01

    The Spallation Neutron Source (SNS), a major new user facility for studies of the structure and dynamics of materials, funded by the US Department of Energy (DOE), is under construction at Oak Ridge National Laboratory (ORNL). Details about the project are available in a recent paper and on the SNS Web site [MRS Bull. 28 (12) (2003) 923]. A Long-Wavelength Target Station (LWTS) [Technical Concepts for a Long-Wavelength Target Station for the Spallation Neutron Source, Argonne National Laboratory Report ANL-02/16, Oak Ridge National Laboratory Report ORNL/SNS-TM-2001/163, November 2002. See also www.pns.anl.gov/related/] will complement the High-Power Target Station (HPTS) facility of the SNS and will build upon the significant investment in the remainder of the installation by providing important new scientific opportunities. For areas of science using the optimized long-wavelength beam lines, the LWTS will at least double the overall scientific capability of the SNS and provide for up to an order of magnitude performance gain over the initial HPTS. The fully equipped SNS has the prospect to offer capabilities for neutron-scattering studies of the structure and dynamics of materials with sensitivity, resolution, dynamic range, and speed that are unparalleled in the world. Preliminary assessments of the performance of the several instruments treated in detail in the body of the paper bear out this expectation. The LWTS concept has been developed in close consultation with the scientific community through a series of workshops and conferences jointly sponsored by DOE's Office of Basic Energy Science and the National Science Foundation. We describe the principal features of the LWTS concept, and provide a preliminary summary of some neutron scattering instruments suited to exploit the unique features of the LWTS. It remains to develop concepts and designs for a full suite of instruments that exploit the capabilities of LWTS, a process that has begun in collaboration

  19. Device for Writing the Time Tail from Spallation Neutron Pulses

    International Nuclear Information System (INIS)

    Langan, P.; Schoenborn, Benno P.; Daemen, L.L.

    2001-01-01

    Recent work at Los Alamos Neutron Science Center (LANSCE), has shown that there are large gains in neutron beam intensity to be made by using coupled moderators at spallation neutron sources. Most of these gains result from broadening the pulse-width in time. However the accompanying longer exponential tail at large emission times can be a problem in that it introduces relatively large beam-related backgrounds at high resolutions. We have designed a device that can reshape the moderated neutron beam by cutting the time-tail so that a sharp time resolution can be re-established without a significant loss in intensity. In this work the basic principles behind the tail-cutter and some initial results of Monte Carlo simulations are described. Unwanted neutrons in the long time-tail are diffracted out of the transmitted neutron beam by a nested stack of aperiodic multi-layers, rocking at the same frequency as the source. Nested aperiodic multi-layers have recently been used at X-ray sources and as band-pass filters in quasi-Laue neutron experiments at reactor neutron sources. Optical devices that rock in synchronization with a pulsed neutron beam are relatively new but are already under construction at LANSCE. The tail-cutter described here is a novel concept that uses existing multi-layer technology in a new way for spallation neutrons. Coupled moderators in combination with beam shaping devices offer the means of increasing flux whilst maintaining a sharp time distribution. A prototype device is being constructed for the protein crystallography station at LANSCE. The protein crystallography station incorporates a water moderator that has been judiciously coupled in order to increase the flux over neutron energies that are important to structural biology (3-80meV). This development in moderator design is particularly important because protein crystallography is flux limited and because conventional ambient water and cold hydrogen moderators do not provide relatively

  20. Reaction-diffusion processes in zero transverse dimensions as toy models for high-energy QCD

    International Nuclear Information System (INIS)

    Armesto, Nestor; Bondarenko, Sergey; Quiroga-Arias, Paloma; Milhano, Jose Guilherme

    2008-01-01

    We examine numerically different zero-dimensional reaction-diffusion processes as candidate toy models for high-energy QCD evolution. Of the models examined-Reggeon Field Theory, Directed Percolation and Reversible Processes-only the latter shows the behaviour commonly expected, namely an increase of the scattering amplitude with increasing rapidity. Further, we find that increasing recombination terms, quantum loops and the heuristic inclusion of a running of the couplings, generically slow down the evolution.

  1. Excitation of long living isomers 107m,109m Ag in the fast neutron inelastic scattering reactions

    International Nuclear Information System (INIS)

    Alpatov, V.G.; Borzakov, S.B.; Chinaeva, V.P

    1999-01-01

    The cross sections for excitation of 107m,109m Ag isomeric states are measured in the reactions of inelastic scattering of reactor fast neutrons. The measurements were performed on the rabbit tube 'Regata' of the IBR-2 reactor (JINR, Dubna). The method consisted in comparing the γ-line intensities of silver isomers with the 103m Rh isomer irradiated in the same neutron flux. The cross sections of 103 Rh are well known in wide range of neutron energy. The measured values are the following: σ( 107m Ag) = 204 ± 18 mb, σ( 109m Ag) = 262 ± 26 mb. The estimate is made of the possible yield of 109m Ag isomeric nuclei if one uses the high-current proton accelerator with heavy target to produce fast neutrons in reactions of spallation. (authors)

  2. Pulsed TRIGA reactor as substitute for long pulse spallation neutron source

    International Nuclear Information System (INIS)

    Whittemore, W.L.

    1999-01-01

    TRIGA reactor cores have been used to demonstrate various pulsing applications. The TRIGA reactor fuel (U-ZrH x ) is very robust especially in pulsing applications. The features required to produce 50 pulses per second have been successfully demonstrated individually, including pulse tests with small diameter fuel rods. A partially optimized core has been evaluated for pulses at 50 Hz with peak pulsed power up to 100 MW and an average power up to 10 MW. Depending on the design, the full width at half power of the individual pulses can range between 2000 μsec to 3000 μsec. Until recently, the relatively long pulses (2000 μsec to 3000 μsec) from a pulsed thermal reactor or a long pulse spallation source (LPSS) have been considered unsuitable for time-of-flight measurements of neutron scattering. More recently considerable attention has been devoted to evaluating the performance of long pulse (1000 to 4000 μs) spallation sources for the same type of neutron measurements originally performed only with short pulses from spallation sources (SPSS). Adequate information is available to permit meaningful comparisons between CW, SPSS, and LPSS neutron sources. Except where extremely high resolution is required (fraction of a percent), which does require short pulses, it is demonstrated that the LPSS source with a 1000 msec or longer pulse length and a repetition rate of 50 to 60 Hz gives results comparable to those from the 60 MW ILL (CW) source. For many of these applications the shorter pulse is not necessarily a disadvantage, but it is not an advantage over the long pulse system. In one study, the conclusion is that a 5 MW 2000 μsec LPSS source improves the capability for structural biology studies of macromolecules by at least a factor of 5 over that achievable with a high flux reactor. Recent studies have identified the advantages and usefulness of long pulse neutron sources. It is evident that the multiple pulse TRIGA reactor can produce pulses comparable to

  3. Investigation of flow asymmetry and instability in the liquid mercury target of the Spallation Neutron Source

    International Nuclear Information System (INIS)

    Pointer, D.; Ruggles, A.; Wendel, M.; Crye, J.

    2000-01-01

    The Spallation Neutron Source (SNS) will utilize a liquid mercury target placed in the path of a high-energy proton beam to produce neutrons for research activities. As the high-energy protons interact with the mercury target, the majority of the beam energy is converted to thermal energy. The liquid mercury must provide sufficient heat transfer to maintain the temperature of the target structure within the thermal limits of the structural materials. Therefore, the behavior of the liquid mercury flow must be characterized in sufficient detail to ensure accurate evaluation of heat transfer in the mercury target. A combination of experimental and computational methods is utilized to characterize the flow in these preliminary analyses. Preliminary studies of the liquid mercury flow in the SNS target indicate that the flow in the exit channel may exhibit multiple recirculation zones, flow asymmetries, and possibly large-scale flow instabilities. While these studies are not conclusive, they serve to focus the efforts of subsequent CFD modeling and experimental programs to better characterize the flow patterns in the SNS mercury target

  4. High energy hadron scattering

    International Nuclear Information System (INIS)

    Johnson, R.C.

    1980-01-01

    High energy and small momentum transfer 2 'yields' 2 hadronic scattering processes are described in the physical framework of particle exchange. Particle production in high energy collisions is considered with emphasis on the features of inclusive reactions though with some remarks on exclusive processes. (U.K.)

  5. Safety concept for spallation target system. JAERI/KEK joint project

    International Nuclear Information System (INIS)

    Kobayashi, K.; Kaminaga, M.; Haga, K.; Kinoshita, H.; Hino, R.

    2001-01-01

    A MW-class mercury target of the spallation target generates much larger amounts of radioactive nuclides than existing spallation neutron sources. To estimate the maximum level of public exposure under the guillotine break of mercury pipelines that is one of the major accidents of the target system, the hazard analyses were carried out by using a transportation model which considers heat transmission of mercury decay heat, diffusion of evaporated radioactive nuclides, etc. In the analyses, mercury, iodine, bromine and noble gas were selected as the effective source term because of their high vapor pressures and activation levels. From the preliminary analytical results obtained under the conservative conditions of 2 m/s of the air velocity around the mercury leakage area, the maximum level of the public exposure was approximately 5.8 x 10 -3 mSv. This level is negligible in comparison with 1 mSV one-year natural radiation exposure. (author)

  6. A few aspects of intermediate energy heavy ion reactions

    International Nuclear Information System (INIS)

    Guet, C.

    1982-10-01

    Some aspects of reactions induced by intermediate energy heavy ions, with a special emphasis of 85 MeV/nucleon 12 C data, are discussed and compared to low energy and relativistic energy features. Transition from mean field to independant nucleon picture is advocated by an increase of nuclear transparency illuminated by reaction cross section estimations. Projectile-like fragment distributions, while demonstrating a typical high energy fragmentation behaviour, exhibit low energy regime distortions. Light fragments, associated to large parallel momentum transfer may result from total explosion. Proton emission is investigated and discussed in terms of opposite models such as thermal equilibrium and nucleon-nucleon scattering. First pion production data are well explained by single nucleon-nucleon inelastic scattering

  7. Beam commission of the high intensity proton source developed at INFN-LNS for the European Spallation Source

    Science.gov (United States)

    Neri, L.; Celona, L.; Gammino, S.; Miraglia, A.; Leonardi, O.; Castro, G.; Torrisi, G.; Mascali, D.; Mazzaglia, M.; Allegra, L.; Amato, A.; Calabrese, G.; Caruso, A.; Chines, F.; Gallo, G.; Longhitano, A.; Manno, G.; Marletta, S.; Maugeri, A.; Passarello, S.; Pastore, G.; Seminara, A.; Spartà, A.; Vinciguerra, S.

    2017-07-01

    At the Istituto Nazionale di Fisica Nucleare - Laboratori Nazionali del Sud (INFN-LNS) the beam commissioning of the high intensity Proton Source for the European Spallation Source (PS-ESS) started in November 2016. Beam stability at high current intensity is one of the most important parameter for the first steps of the ongoing commissioning. Promising results were obtained since the first source start with a 6 mm diameter extraction hole. The increase of the extraction hole to 8 mm allowed improving PS-ESS performances and obtaining the values required by the ESS accelerator. In this work, extracted beam current characteristics together with Doppler shift and emittance measurements are presented, as well as the description of the next phases before the installation at ESS in Lund.

  8. Contribution to the phenomenological study of two-body reactions at high energy; Contribution a l'etude phenomenologique des reactions a deux corps a haute energie

    Energy Technology Data Exchange (ETDEWEB)

    Cohen-Tannoudji, G [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires

    1968-07-01

    A phenomenological model suited for the description of arbitrary two-body reactions at high energies is presented and applied to the analysis of {pi} - nucleon, K - nucleon, et K-bar - nucleon scattering.The idea is that the Regge-pole model does not take into account the whole content of the unitarity relation and has to be modified, as is currently done in one-particle exchange models, so that it may include absorptive corrections.In terms of a rather economical set of free parameters,we obtain a satisfactory agreement with all available data, including the recent evidence for a nonvanishing polarization in {pi}{sup -} p {pi}{sup 0} n reaction. We then reinterpret our parametrization of the amplitudes in terms of poles and branch points in the complex angular-momentum plane for the crossed channel. (author) [French] Un modele phenomenologique adapte a la description des reactions a deux corps a haute energie est presente et applique a l'analyse des diffusions {pi} - nucleon, K - nucleon, et K-bar - nucleon. L'idee essentielle est que le modele d'echange de poles de Regge ne tient pas compte du contenu total de la relation d'unitarite et doit etre modifie, comme cela a ete propose dans le cas de l'echange de particules, de facon a tenir compte de corrections de type absortif. Au moyen d'un ensemble relativement economique de parametres libres nous obtenons un accord satisfaisant avec tous les resultats disponibles, y compris l'existence recemment mise en evidence d'une polarisation non nulle dans la reaction {pi}{sup -} p {pi}{sup 0} n. Nous interpretons notre fa n d'ecrire les amplitudes au moyen de poles et de points de branchement dans le plan complexe du moment angulaire pour la voie croisee. (auteur)

  9. Some results of applied spallation physics research at Los Alamos

    International Nuclear Information System (INIS)

    Russell, G.J.; Gilmore, J.S.

    1983-01-01

    At the Los Alamos National Laboratory, we have an active effort in the general area of Applied Spallation Physics Research. The main emphasis of this activity has been on obtaining basic data relevant to spallation neutron source development, accelerator breeder technology, and validation of computer codes used in these applications. We present here an overview of our research effort and show some measured and calculated results of differential and clean integral experiments

  10. Improvement of the spallation-reaction simulation code by considering both the high-momentum intranuclear nucleons and the preequilibrium process

    International Nuclear Information System (INIS)

    Ishibashi, K.; Miura, Y.; Sakae, T.

    1990-01-01

    In the present study, intranuclear nucleons with a high momentum are introduced into intranuclear cascade calculation, and the preequilibrium effects are considered at the end of the cascade process. The improvements made in the HETC (High Energy Transport Code) are outlined, focusing on intranuclear nucleons with a high momentum, and termination of the intranuclear cascade process. Discussion is made of the cutoff energy, and Monte Carlo calculations based on an excitation model are presented and analyzed. The experimental high energy neutrons in the backward direction are successfully reproduced. The preequilibrium effect is considered in a local manner, and this is introduced as a simple probability density function for terminating the intranuclear cascade process. The resultant neutron spectra reproduce the shoulders of the experimental data in the region of 20 to 50 MeV. The exciton model is coded with a Monte Carlo algorithm. The results of the exciton model calculation is not so appreciable except for intermediate energy neutrons in the backward direction. (N.K.)

  11. Reaction-rate coefficients, high-energy ions slowing-down, and power balance in a tokamak fusion reactor plasma

    International Nuclear Information System (INIS)

    Tone, Tatsuzo

    1978-07-01

    Described are the reactivity coefficient of D-T fusion reaction, slowing-down processes of deuterons injected with high energy and 3.52 MeV alpha particles generated in D-T reaction, and the power balance in a Tokamak reactor plasma. Most of the results were obtained in the first preliminary design of JAERI Experimental Fusion Reactor (JXFR) driven with stationary neutral beam injection. A manual of numerical computation program ''BALTOK'' developed for the calculations is given in the appendix. (auth.)

  12. Study of steady-state heat transfer with various large beam intensities in ADS windowless spallation target

    International Nuclear Information System (INIS)

    Liu, Jie; Gao, Lei; Tong, Jian-fei; Mehmood, Irfan; Lu, Wen-qiang

    2015-01-01

    Thermal hydraulics of spallation target, which is regarded as the ‘heart’ of the accelerator driven system (ADS), is very complicated due to the flow of the heavy liquid metal, spallation reaction and the coupling. In this paper, the steady-state temperature distribution, based on the flow pattern and the heat deposition, in the windowless spallation target with various large beam intensities from 10 mA to 40 mA is obtained to be in line with the development of ADS in China. The results show that the shape of temperature distribution is the same as broken wing of the butterfly but the temperature gradient and the maximum temperature vary in proportion with beam intensity. The variation of temperature gradient in different zones is also used to figure out the effect of large beam intensity. It has been found that large radial and axial temperature gradient leads to large temperature gradient on the wall. This may cause extremely large thermal stresses which leads to structural material damage. The results may be applied to the future design and optimization of ADS in China. - Highlights: • Shape of temperature distribution is the same but temperature gradient and maximum temperature vary with intensity. • The variation of temperature gradient in different zones reveals the effect of large beam intensity. • Large radial and axial temperature gradient leads to large temperature gradient on the wall

  13. Resolution of the VESUVIO spectrometer for High-energy Inelastic Neutron Scattering experiments

    Energy Technology Data Exchange (ETDEWEB)

    Imberti, S. [Universita degli Studi di Roma Tre, Dipartimento di Fisica ' E.Amaldi' , Rome (Italy) and CNR-INFM, Rome (Italy)]. E-mail: silvia.imberti@roma2.infn.it; Andreani, C. [Universita degli Studi di Roma Tor Vergata, Dipartimento di Fisica, Roma 60133 (Italy); CNR-INFM, Rome (Italy); Garbuio, V. [Universita degli Studi di Roma Tor Vergata, Dipartimento di Fisica, Roma 60133 (Italy); CNR-INFM, Rome (Italy); Gorini, G. [Universita degli Studi di Milano-Bicocca, Dipartimento di Fisica ' G.Occhialini' , Milan (Italy); CNR-INFM, Milan (Italy); Pietropaolo, A. [Universita degli Studi di Roma Tor Vergata, Dipartimento di Fisica, Roma 60133 (Italy); CNR-INFM, Rome (Italy); Senesi, R. [Universita degli Studi di Roma Tor Vergata, Dipartimento di Fisica, Roma 60133 (Italy); CNR-INFM, Rome (Italy); Tardocchi, M. [Universita degli Studi di Milano-Bicocca, Dipartimento di Fisica ' G.Occhialini' , Milan (Italy); CNR-INFM, Milan (Italy)

    2005-11-01

    New perspectives for epithermal neutron spectroscopy have been opened up as a result of the development of the Resonance Detector and its use on inverse geometry time-of-flight spectrometers at spallation sources. A special application of the Resonance Detector is the Very Low Angle Detector Bank (VLAD) for the VESUVIO spectrometer at ISIS, operating in the angular range 1 deg. <2{theta}<5 deg. This equipment allows High-energy Inelastic Neutron Scattering (HINS) measurements to be performed in the (q,{omega}) kinematical region at low wavevector (q<10A{sup -1}) and high energy (unlimited) transfer -bar {omega}>500meV, a regime so far inaccessible to experimental studies on condensed matter systems. The HINS measurements complement the Deep Inelastic Neutron Scattering (DINS) measurements performed on VESUVIO in the high wavevector q(20A{sup -1}high energy transfer (-bar {omega}>1eV), where the short-time single-particle dynamics can be sampled. This paper will revise the main components of the resolution for HINS measurements of VESUVIO. Instrument performances and examples of applications for neutron scattering processes at high energy and at low wavevector transfer are discussed.

  14. Pulsed spallation Neutron Sources

    International Nuclear Information System (INIS)

    Carpenter, J.M.

    1994-01-01

    This paper reviews the early history of pulsed spallation neutron source development at Argonne and provides an overview of existing sources world wide. A number of proposals for machines more powerful than currently exist are under development, which are briefly described. The author reviews the status of the Intense Pulsed Neutron Source, its instrumentation, and its user program, and provides a few examples of applications in fundamental condensed matter physics, materials science and technology

  15. Pulsed spallation neutron sources

    International Nuclear Information System (INIS)

    Carpenter, J.M.

    1996-01-01

    This paper reviews the early history of pulsed spallation neutron source development ar Argonne and provides an overview of existing sources world wide. A number of proposals for machines more powerful than currently exist are under development, which are briefly described. The author reviews the status of the Intense Pulsed Neutron Source, its instrumentation, and its user program, and provide a few examples of applications in fundamental condensed matter physics, materials science and technology

  16. THE SPALLATION NEUTRON SOURCE PROJECT - PHYSICAL CHALLENGES.

    Energy Technology Data Exchange (ETDEWEB)

    WEI,J.

    2002-06-03

    The Spallation Neutron Source (SNS) is designed to reach an average proton beam power of 1.4 MW for pulsed neutron production. This paper summarizes design aspects and physical challenges to the project.

  17. INFLUENCE OF MICROSTRUCTURAL ANISOTROPY ON THE SPALLATION OF 1080 EUTECTOID STEEL

    International Nuclear Information System (INIS)

    GRAY, G.T.; LOPEZ, M.F.

    2001-01-01

    While the influence of crystallographic texture on elastic and plastic constitutive response has seen extensive investigation in recent years, the influence of texture on the dynamic fracture of engineering materials remains less extensively explored. In particular, the influence of anisotropy, both textural and morphological, on the spallation behavior of materials remains poorly quantified. In this study, the spallation response of 1080-steel has been studied as a function of microstructural morphological anisotropy. In this study the influence of elongated MnS stringers, resident within a crystallographically isotropic eutectoid steel, on the spallation response of 1080 steel was investigated. That of a fully-pearlitic 1080 steel loaded to 5 GPa was found to be dominated by the heterogeneous nucleation of damage normal and orthogonal to the MnS stringers. Delamination between the matrix pearlitic microstructure and the MnS stringers was seen to correlate to a significantly lower pull-back signal during transverse loading than to that parallel to the stringer axis. The ''pull-back'' signals and post-spallation metallographic observations are discussed with reference to the influence of microstructural anisotropy on void nucleation and growth

  18. Design and implementation of low-Q diffractometers at spallation sources

    International Nuclear Information System (INIS)

    Seeger, P.A.; Hjelm, R.P.

    1993-01-01

    Low-Q diffractometers at spallation sources that use time of flight methods have been successfully implemented at several facilities, including the Los Alamos Neutron Scattering Center. The proposal to build new, more powerful, advanced spallation sources using advanced moderator concepts will provide luminosity greater than 20 times the brightest spallation source available today. These developments provide opportunity and challenge to expand the capabilities of present instruments with new designs. The authors review the use of time of flight for low-Q measurements and introduce new designs to extend the capabilities of present-day instruments. They introduce Monte Carlo methods to optimize design and simulate the performance of these instruments. The expected performance of the new instruments are compared to present day pulsed source- and reactor-based small-angle neutron scattering instruments. They review some of the new developments that will be needed to use the power of brighter sources effectively

  19. Multipolarity analysis for 14C high-energy resonance populated by (18O,16O) two-neutron transfer reaction

    International Nuclear Information System (INIS)

    Carbone, D.; Cavallaro, M.; Bondì, M.; Agodi, C.; Cunsolo, A.; Cappuzzello, F.; Azaiez, F.; Franchoo, S.; Khan, E.; Bonaccorso, A.; Fortunato, L.; Foti, A.; Linares, R.; Lubian, J.; Scarpaci, J. A.; Vitturi, A.

    2015-01-01

    The 12 C( 18 O, 16 O) 14 C reaction at 84 MeV incident energy has been explored up to high excitation energy of the residual nucleus thanks to the use of the MAGNEX spectrometer to detect the ejectiles. In the region above the two-neutron separation energy, a resonance has been observed at 16.9 MeV. A multipolarity analysis of the cross section angular distribution indicates an L = 0 character for such a transition

  20. Facility for fast neutron irradiation tests of electronics at the ISIS spallation neutron source

    International Nuclear Information System (INIS)

    Andreani, C.; Pietropaolo, A.; Salsano, A.; Gorini, G.; Tardocchi, M.; Paccagnella, A.; Gerardin, S.; Frost, C. D.; Ansell, S.; Platt, S. P.

    2008-01-01

    The VESUVIO beam line at the ISIS spallation neutron source was set up for neutron irradiation tests in the neutron energy range above 10 MeV. The neutron flux and energy spectrum were shown, in benchmark activation measurements, to provide a neutron spectrum similar to the ambient one at sea level, but with an enhancement in intensity of a factor of 10 7 . Such conditions are suitable for accelerated testing of electronic components, as was demonstrated here by measurements of soft error rates in recent technology field programable gate arrays

  1. Status of Cea spallation modules for ads

    International Nuclear Information System (INIS)

    Enderle, R.; Poitevin, Y.; Deffain, J.P.; Bergeron, J.

    2001-01-01

    In the framework of CEA studies on ADS dedicated to waste transmutation, a liquid metal reference concept and an alternative solid target have been evaluated to produce neutrons inside the spallation module. This work examines the design (neutronic, thermohydraulic and mechanical aspects) and the performances of both options. It is shown that a liquid Pb-Bi target offers more possibilities regarding to high protons current densities (possible industrial extrapolation) but that a solid target made with tungsten particles offers also interesting ability to create a neutrons flux appropriated (strong spectrum and flat axial distribution) to an sub-critical core dedicated to incineration. (author)

  2. Differential production cross sections of multiply charged fragments in 800 MeV proton-induced spallation of carbon, aluminum, and nickel

    International Nuclear Information System (INIS)

    Luckstead, S.C.

    1978-09-01

    Differential production cross sections for multiply charged fragments from 800-MeV proton-induced spallation of 12 C, 27 Al, and natural Ni were measured at 30 and 90 degrees. The ion fragments were identified by use of time-of-flight, ΔE--E detector telescope capable of complete particle identification for energies as low as .25 MeV/nucleon. The very short ranges of the particles of interest required the construction of very thin detectors with minimal deadlayer material. The time-pick-off detectors and gas ionization chamber developed are unique, and represent the state-of-the-art in fast timing for time-of-flight measurements and in construction of thin detectors. The resolutions achieved allowed the cross sections of 3 He, 4 He, 6 Li, 7 Li, 7 Be, 9 Be, 10 Be, 10 B, 11 B, 11 C, 12 C, and 13 C to be determined, along with those of nitrogen and oxygen without isotope separation. The cross sections were found to have weak angular dependence. Consequently, pseudo cross sections were calculated from the 90 0 data by integrating the differential cross sections from 0 to 25 MeV for each product and multiplying by 4π. Pseudo theoretical cross sections were similarly calculated from theoretical differential cross sections. These differential cross sections were calculated by use of a Monte Carlo computer code which incorporated the cascade-evaporation model of high-energy nuclear reactions. Implications are drawn for modifications of the model. The results suggest reducing the transparency of the struck nucleus to pions produced in the cascade stage of the reaction model in order that a higher excitation energy be left for the evaporation stage. Also, there is some evidence that evaporations of nuclear aggregates more massive than 4 He occur. Inclusion of such evaporations should improve the model. 82 figures, 1 table

  3. Background studies of high energy γ rays from (n,γ) reactions in the CANDLES experiment

    Science.gov (United States)

    Nakajima, K.; Iida, T.; Akutagawa, K.; Batpurev, T.; Chan, W. M.; Dokaku, F.; Fushimi, K.; Kakubata, H.; Kanagawa, K.; Katagiri, S.; Kawasaki, K.; Khai, B. T.; Kino, H.; Kinoshita, E.; Kishimoto, T.; Hazama, R.; Hiraoka, H.; Hiyama, T.; Ishikawa, M.; Li, X.; Maeda, T.; Matsuoka, K.; Moser, M.; Nomachi, M.; Ogawa, I.; Ohata, T.; Sato, H.; Shamoto, K.; Shimada, M.; Shokati, M.; Takahashi, N.; Takemoto, Y.; Takihira, Y.; Tamagawa, Y.; Tozawa, M.; Teranishi, K.; Tetsuno, K.; Trang, V. T. T.; Tsuzuki, M.; Umehara, S.; Wang, W.; Yoshida, S.; Yotsunaga, N.

    2018-07-01

    High energy γ rays with several MeV produced by (n,γ) reactions can be a trouble for low background measurements in the underground laboratories such as double beta decay experiments. In the CANDLES project, which aimed to observe the neutrino-less double beta decay from 48Ca, γ rays caused by (n,γ) reactions were found to be the most significant background. The profile of the background was studied by measurements with a neutron source and a simulation with a validity check of neutron processes in Geant4. The observed spectrum of γ rays from (n,γ) reactions was well reproduced by the simulated spectra, which were originated from the surrounding rock and a detector tank made of stainless steel. The environmental neutron flux was derived by the observed event rate of γ rays from (n,γ) reactions using the simulation. The thermal and non-thermal neutron flux were found to be (1.3 ± 0.6) ×10-6 cm-2s-1 and (1.1 ± 0.5) ×10-5 cm-2s-1 , respectively. It is necessary to install an additional shield to reduce the background from (n,γ) reaction to the required level.

  4. Low Energy Nuclear Reactions: 2007 Update

    Science.gov (United States)

    Krivit, Steven B.

    2007-03-01

    This paper presents an overview of low energy nuclear reactions, a subset of the field of condensed matter nuclear science. Condensed matter nuclear science studies nuclear effects in and/or on condensed matter, including low energy nuclear reactions, an entirely new branch of science that gained widespread attention and notoriety beginning in 1989 with the announcement of a previously unrecognized source of energy by Martin Fleischmann and Stanley Pons that came to be known as cold fusion. Two branches of LENR are recognized. The first includes a set of reactions like those observed by Fleischmann and Pons that use palladium and deuterium and yield excess heat and helium-4. Numerous mechanisms have been proposed to explain these reactions, however there is no consensus for, or general acceptance of, any of the theories. The claim of fusion is still considered speculative and, as such, is not an ideal term for this work. The other branch is a wide assortment of nuclear reactions that may occur with either hydrogen or deuterium. Anomalous nuclear transmutations are reported that involve light as well as heavy elements. The significant questions that face this field of research are: 1) Are LENRs a genuine nuclear reaction? 2) If so, is there a release of excess energy? 3) If there is, is the energy release cost-effective?

  5. High energy physics and nuclear structure

    International Nuclear Information System (INIS)

    Measday, D.F.; Thomas, A.W.

    1980-01-01

    These proceedings contain the papers presented at the named conference. These concern eletromagnetic interactions, weak interactions, strong interactions at intermediate energy, pion reactions, proton reactions, strong interactions at high energy, as well as new facilities and applications. See hints under the relevant topics. (HSI)

  6. Peripheral Ar induced reactions at 44MeV/u. Similarities and deviations with respect to a high energy fragmentation process

    International Nuclear Information System (INIS)

    Borrel, V.; Guerreau, D.; Galin, J.; Gatty, B.; Jacquet, D.; Tarrago, X.

    1983-01-01

    Peripheral Ar reactions induced on 58 Ni at GANIL at 44 MeV/u have been analyzed in the framework of the high energy fragmentation model. Several deviations from this model have been interpreted as due to the persistence of some collective effects at this intermediate energy

  7. Laser-irradiated thermodynamic behaviors of spallation and recombination at solid-state interface

    International Nuclear Information System (INIS)

    Lai, H.-Y.; Huang, P.-H.

    2008-01-01

    A microscopic insight of interfacial spallation and recombination behaviors at multilayer thin-film interface induced by incident femtosecond pulsed laser is presented in this paper. Such two different aforementioned behaviors are investigated via the thermodynamic trajectories obtained by using standard Lennard-Jones (L-J) molecular dynamics (MD) simulation. Based on the simulation results, the interfacial damages of multilayer thin film are dominated by a critical threshold that induces an extraordinary expansive dynamics and phase transitions leading to the structural softened and tensile spallation at interface. The critical damage threshold is evaluated at around 8.5 J/m 2 which governs the possible occurrence of two different regimes, i.e. interfacial spallaiton and recombination. In interfacial damage region, quasi-isothermal thermodynamic trajectories can be observed after the interfacial spallation occurs. Moreover, the result of thermodynamic trajectories analyses indicates that, the relaxation of pressure wave may cause the over-heated interfacial zone to reduce volumetric density, thus leading to structural softness and even weaken interfacial structural strength. The crucial effect leading to the phenomenon of low tension spallation is identified

  8. The 14N(p, γ)15O reaction studied at low and high beam energy

    International Nuclear Information System (INIS)

    Marta, Michele

    2012-01-01

    The Bethe-Weizsaecker cycle consists of a set of nuclear reactions that convert hydrogen into helium and release energy in the stars. It determines the luminosity of low-metal stars at their turn-off from the main-sequence in the Hertzsprung-Russel diagram, so its rate enters the calculation of the globular clusters' age, an independent lower limit on the age of the universe. The cycle contributes less than 1% to our Sun's luminosity, but it produces neutrinos that can in principle be measured on Earth in underground experiments and bring direct information of the physical conditions in the solar core, provided that the nuclear reaction rate is known with sufficient precision. The 14 N(p,γ) 15 O reaction is the slowest reaction of the Bethe-Weizsaecker cycle and establishes its rate. Its cross section is the sum of the contributions by capture to different excited levels and to the ground state in 15 O. Recent experiments studied the region of the resonance at E p = 278 keV. Only one modern data set from an experiment performed in 1987 is available for the high-energy domain. Both energy ranges are needed to constrain the fit of the excitation function in the R-matrix framework and to obtain a reliable extrapolated S-factor at the very low astrophysical energies. The present research work studied the 14 N(p,γ) 15 O reaction in the LUNA (Laboratory for Underground Nuclear Astrophysics) underground facility at three proton energies 0.36, 0.38, 0.40MeV, and in Dresden in the energy range E p = 0.6 - 2MeV. In both cases, an intense proton beam was sent on solid titanium nitride sputtered targets, and the prompt photons emitted from the reaction were detected with germanium detectors. At LUNA, a composite germanium detector was used. This enabled a measurement with dramatically reduced summing corrections with respect to previous studies. The cross sections for capture to the ground state and to the excited states at 5181, 6172, and 6792 keV in 15 O have been

  9. Neutron scattering instruments for the Spallation Neutron Source (SNS)

    International Nuclear Information System (INIS)

    Crawford, R.K.; Fornek, T.; Herwig, K.W.

    1998-01-01

    The Spallation Neutron Source (SNS) is a 1 MW pulsed spallation source for neutron scattering planned for construction at Oak Ridge National Laboratory. This facility is being designed as a 5-laboratory collaboration project. This paper addresses the proposed facility layout, the process for selection and construction of neutron scattering instruments at the SNS, the initial planning done on the basis of a reference set of ten instruments, and the plans for research and development (R and D) to support construction of the first ten instruments and to establish the infrastructure to support later development and construction of additional instruments

  10. Dynamics of high energy reactions

    International Nuclear Information System (INIS)

    Field, R.D.

    1979-01-01

    During last several years, a new framework to describe strong interaction physics has emerged, i.e. quantum chromodynamics (QCD). It is the simplest field theory which incorporates color-dependent force among quarks. This force is generated by the exchange of colored vector gluons coupled to the quarks in gauge-invariant manner. The theory is closely related to the most successful quantum field theory, QED, and the only but very important difference is the gauge group involved. Although the theory is well defined, precisely what it predicts is not yet clearly known. However, at very high energy or momentum transfer Q, the effective coupling between quarks and gluons decreases toward zero with increasing Q 2 , and the calculation of a process involving high Q 2 is possible by the use of perturbation theory. In this paper, many applications of QCD to the processes involving high momentum transfer are examined. The effective coupling resulting from strong interaction between quarks and gluons, the scale violation in deep inelastic lepton scattering, large mass muon pair production, quark and gluon fragmentation functions, large transverse momentum meson and jet production in hadron-hadron collision, and the search for three-jet events are discussed. (Kako, I.)

  11. Spallation impact analysis of plutonium storage container at K-Area

    International Nuclear Information System (INIS)

    Gong, C.

    2000-01-01

    A 100-pound concrete block falls 55-foot from ceiling spallation upon the top of the 9975 shipping package. This finite element analysis aims to evaluate the dynamic impact from the spallation upon the packaging. The geometric configuration of the packaging is meticulously modeled in detail. However, the drum is eliminated and the fiberboard with radius greater than 5.6 inches is conservatively omitted. The primary containment vessel and 3013 container were not included to simplify the model. The concrete block is modeled as a rigid body. The material properties are conservatively selected. The final results indicate that the secondary containment vessel is intact during this spallation impact. Consequently the primary containment vessel and 3013 container would not experience damage and containment is maintained. The secondary containment vessel protects the primary containment vessel from the dynamic impact. The top fiberboard is compressed from 3.5 inches to 0.875 inches will eventually recover to 1.8 inches according to tests performed at Savannah River Technology Center (SRTC)

  12. The 56Fe(n,x α) reaction from threshold to 30 MeV

    International Nuclear Information System (INIS)

    Sterbenz, S.M.; Young, P.G.; Bateman, F.B.

    1994-01-01

    Alpha-particle emission in neutron reactions with 56 Fe has been studied from threshold to over 30 MeV using the spallation neutron source at WNR/LAMPF. Alpha-particle production cross sections, spectra, and angular distributions were measured at scattering angles of 30, 60, 90, and 135 degrees using detector telescopes consisting of a low-pressure gas proportional counter and a large area silicon detector. Time-of-flight techniques with a 10-meter flight path were used to deduce the incident neutron energies. Our results are compared with literature values and with several theoretical calculations

  13. Application of a controlled swirl in the XT-ADS spallation target

    International Nuclear Information System (INIS)

    Roelofs, F.; Siccama, N. B.; Jeanmart, H.; Tichelen, K. V.; Dierckx, M.; Schuurmans, P.

    2008-01-01

    Within the EUROTRANS project, a windowless spallation target is designed and assessed in which there is direct contact between the proton beamline vacuum from the accelerator and a lead-bismuth free surface flow. Windowless spallation targets, which are designed by SCK.CEN, based on their experience for the MYRRHA concept, are experimentally examined in a well instrumented water-loop at UCL. The design work and the experimental campaign are supported by numerical simulations which are performed at NRG. In the current paper, the application of a mild swirl in the windowless spallation target is assessed. For this purpose, SCK.CEN has designed and fabricate, a spallation target in which a controlled swirl is introduced in the annular feeder of the target nozzle. An experimental programme is performed at UCL in their water-loop to evaluate various swirl strengths in one specific target nozzle design. Prior to the experimental programme, numerical simulations were performed at NRG assessing the influence of various swirl strengths on the free surface behaviour. Experimental and numerical results show that a mild swirl stabilizes the free surface and also indicate that applying a stronger swirl leads to undesired free surface behaviour, ultimately leading to a strong vortex in the central downcomer. (authors)

  14. X-ray microtomography study of the spallation response in Ta-W

    Science.gov (United States)

    McDonald, Samuel; Cotton, Matthew; Millett, Jeremy; Bourne, Neil; Withers, Philip

    2013-06-01

    The response of metallic materials to high strain-rate (impact) loading is of interest to a number of communities. Traditionally, the largest driver has been the military, in its need to understand armour and resistance to ballistic attack. More recently, industries such as aerospace (foreign object damage, bird strike, etc.), automotive (crash-worthiness) and satellite protection (orbital debris) have all appreciated the necessity of such information. It is therefore important to understand the dynamic tensile or spallation response, and in particular to be able to observe in three-dimensions, and in a non-invasive manner, the physical damage present in the spalled region post-impact. The current study presents plate impact experiments investigating the spallation damage response of recovered targets of the tantalum alloy Ta-2.5%W. Using X-ray microtomography the damage resulting from differing impact conditions (impact velocity/stress, pulse duration) is compared and characterised in 3-D. Combined with free surface velocity measurements, the tensile failure mechanisms during dynamic loading have been identified.

  15. Radiation problems expected for the German spallation neutron source

    International Nuclear Information System (INIS)

    Goebel, K.

    1981-01-01

    The German project for the construction of a Spallation Neutron Source with high proton beam power (5.5 MW) will have to cope with a number of radiation problems. The present report describes these problems and proposes solutions for keeping exposures for the staff and release of activity and radiation into the environment as low as reasonably achievable. It is shown that the strict requirements of the German radiation protection regulations can be met. The main problem will be the exposure of maintenance personnel to remanent gamma radiation, as is the case at existing proton accelerators. Closed ventilation and cooling systems will reduce the release of (mainly short-lived) activity to acceptable levels. Shielding requirements for different sections are discussed, and it is demonstrated by calculations and extrapolations from experiments that fence-post doses well below 150 mrem/y can be obtained at distances of the order of 100 metres from the principal source points. The radiation protection system proposed for the Spallation Neutron Source is discussed, in particular the needs for monitor systems and a central radiation protection data base and alarm system. (orig.)

  16. Neutron-induced complex reaction analysis with 3D nuclear track simulation

    International Nuclear Information System (INIS)

    Sajo-Bohus, L.; Palfalvi, J.K.; Akatov, Yu.; Arevalo, O.; Greaves, E.D.; Nemeth, P.; Palacios, D.; Szabo, J.; Eoerdoegh, I.

    2005-01-01

    Complex (multiple) etched tracks are analysed through digitised images and 3D simulation by a purpose-built algorithm. From a binary track image an unfolding procedure is followed to generate a 3D track model, from which several track parameters are estimated. The method presented here allows the deposited energy, that originated from particle fragmentation or carbon spallation by means of induced tracks in commercially available PADC detectors, to be estimated. Results of evaluated nuclear tracks related to 12 C (n,3αn ' ) reaction are presented here. The detectors were exposed on the ISS in 2001

  17. Spallation-based science and technology and associated nuclear data requirements

    International Nuclear Information System (INIS)

    Bowman, C.D.; Lisowski, P.W.; Arthur, E.D.

    1990-01-01

    Rapid advances in accelerator technology in recent years promise average proton beam currents as high as 250 mA with energies greater than one GeV. Such an accelerator could produce very high intensities of neutrons and other nuclear particles thus opening up new areas of science and technology. An example is the efficient burning of transuranic and fission product waste. With such a spallation-burner it appears that high-level waste might be converted to low-level waste on a time scale comparable to the human lifespan at a reasonable additional cost for electric power generation. The emphasis of this paper is on the design of a high power proton target for neutron production, on the nuclear data needed to operate this target safely and effectively, and on data requirements for transmutation. It is suggested that a pilot facility consisting of a 1.6 GeV accelerator and target operating at 25 ma is the next major step in developing this technology. Bursts of protons near the terawatt level might also be generated using such an accelerator with a proton accumulator ring. Research prospects based on such proton bursts are briefly described. The status of established nuclear data needs and of accelerator-based sources for nuclear data measurements is reviewed. (author)

  18. Characteristics of the WNR: a pulsed spallation neutron source

    International Nuclear Information System (INIS)

    Russell, G.J.; Lisowski, P.W.; Howe, S.D.; King, N.S.P.; Meier, M.M.

    1982-01-01

    The Weapons Neutron Research facility (WNR) is a pulsed spallation neutron source in operation at the Los Alamos National Laboratory. The WNR uses part of the 800-MeV proton beam from the Clinton P. Anderson Meson Physics Facility accelerator. By choosing different target and moderator configurations and varying the proton pulse structure, the WNR can provide a white neutron source spanning the energy range from a few MeV to 800 MeV. The neutron spectrum from a bare target has been measured and is compared with predictions using an Intranuclear Cascade model coupled to a Monte Carlo transport code. Calculations and measurements of the neutronics of WNR target-moderator assemblies are presented

  19. Sulfur and Moisture Effects on Alumina Scale and TBC Spallation

    Science.gov (United States)

    Smialek, James L.

    2007-01-01

    cause is related to a hydrogen embrittlement reaction: Al alloy + 3 H2O = Al(OH)3 + 3H(+) + 3e(-). This mechanism is derived from an analogous moisture-induced hydrogen embrittlement mechanism originally shown for Ni3Al and FeAl intermetallics. Consequently, a cathodic hydrogen charging technique was used to demonstrate that electrolytic de-scaling occurs for these otherwise adherent alumina scales formed on Y-doped Rene'N5, in support of hydrogen effects. Finally, some TBC observations are discussed in light of all of the above. Plasma sprayed 8YSZ coatings, produced on PWA1484 without a bond coat, were found to survive more than 1000 1-hr cycles at 1100 C when desulfurized to below 0.1 ppmw. At higher sulfur (1.2 ppmw) levels, moisture sensitivity and delayed TBC failure, referred to as Desk Top Spallation, occurred at just 200 hr. Despite a large degree of scatter, a factor of 5 in life improvement is indicated for desulfurized samples in cyclic furnace tests, confirming the beneficial effect of low sulfur alloys on model TBC systems. (DTS and moisture effects are also observed on commercially applied PVD 7YSZ coatings on Rene'N5+Y with Pt-aluminide bond coats). These types of catastrophic failure were subverted on the model system by segmenting the substrate into a network of 0.010 high ribs, spaced in. apart, prior to plasma spraying. No failures occurred after 1000 cycles at 1150 C or after 2000 cycles at 1100 C, even after water immersion. The benefit is described in terms of elasticity models and a critical buckling stress.

  20. Synchrotron-driven spallation sources

    CERN Document Server

    Bryant, P J

    1996-01-01

    The use of synchrotrons for pulsed neutron spallation sources is an example of scientific and technological spin-off from the accelerator development for particle physics. Accelerator-driven sources provide an alternative to the continuous-flux, nuclear reactors that currently furnish the majority of neutrons for research and development. Although the present demand for neutrons can be adequately met by the existing reactors, this situation is unlikely to continue due to the increasing severity of safety regulations and the declared policies of many countries to close down their reactors within the next decade or so. Since the demand for neutrons as a research tool is, in any case,expected to grow, there has been a corresponding interest in sources that are synchrotron-driven or linac-driven with a pulse compression ring and currently several design studies are being made. These accelerator-driven sources also have the advantage of a time structure with a high peak neutron flux. The basic requirement is for a...

  1. Surface Laser Scanning Measurements for the n_TOF spallation target

    CERN Document Server

    Vlachoudis, V; Cennini, P; Lebbos, E; Lettry, J

    2010-01-01

    The n_TOF spallation target is made of pure lead immersed into cooling water. The target was operating normally from 2001 until august 2004, when an increased transfer of radioactive products from the spallation target to the cooling circuit has been observed. The target was considered damaged by the safety commission (SC/RP), and an investigation campaign started to verify the actual status of the target. According to FLUKA and Ansys calculations the target was working in the elastoplastic regime of the lead material, therefore a deformation might be expected. The present paper describes a laser photographic method and the results of a possible such deformation. The target had a surface activity of the order of 20 mSv/h, therefore we were forced to perform the measurement from distance. The used method, is based on a linelaser and a high resolution digital camera for retrieving the 3D position of the surface of the lead target. Similar methods are used in the film industry and animation studios for scanning ...

  2. 32S-induced reactions at 10 MeV/u bombarding energy

    International Nuclear Information System (INIS)

    Betz, J.; Graef, H.; Novotny, R.; Pelte, D.; Winkler, U.

    1983-01-01

    The deep-inelastic processes of the reactions 32 S+ 28 Si, sup(nat)S, 40 Ca, 58 Ni, 74 Ge are studied at 10 MeV/u bombarding energy employing a kinematical coincidence spectrometer. From the measured energies, momenta, masses and atomic numbers of two heavy fragments the corresponding parameters for the unobserved reaction products and the reaction Q-values are deduced. It is found that the reactions generally show the pattern of a normal deep-inelastic process which is followed by the evaporation of several light particles. But with much less intensities other processes also seem to occur: three-fragment excit channels and incomplete energy damping which is correlated with the emission of a few light particles of high momenta. (orig.)

  3. Calculation of reaction energies and adiabatic temperatures for waste tank reactions

    International Nuclear Information System (INIS)

    Burger, L.L.

    1995-10-01

    Continual concern has been expressed over potentially hazardous exothermic reactions that might occur in Hanford Site underground waste storage tanks. These tanks contain many different oxidizable compounds covering a wide range of concentrations. The chemical hazards are a function of several interrelated factors, including the amount of energy (heat) produced, how fast it is produced, and the thermal absorption and heat transfer properties of the system. The reaction path(s) will determine the amount of energy produced and kinetics will determine the rate that it is produced. The tanks also contain many inorganic compounds inert to oxidation. These compounds act as diluents and can inhibit exothermic reactions because of their heat capacity and thus, in contrast to the oxidizable compounds, provide mitigation of hazardous reactions. In this report the energy that may be released when various organic and inorganic compounds react is computed as a function of the reaction-mix composition and the temperature. The enthalpy, or integrated heat capacity, of these compounds and various reaction products is presented as a function of temperature; the enthalpy of a given mixture can then be equated to the energy release from various reactions to predict the maximum temperature which may be reached. This is estimated for several different compositions. Alternatively, the amounts of various diluents required to prevent the temperature from reaching a critical value can be estimated. Reactions taking different paths, forming different products such as N 2 O in place of N 2 are also considered, as are reactions where an excess of caustic is present. Oxidants other than nitrate and nitrite are considered briefly

  4. Calculation of reaction energies and adiabatic temperatures for waste tank reactions

    Energy Technology Data Exchange (ETDEWEB)

    Burger, L.L.

    1995-10-01

    Continual concern has been expressed over potentially hazardous exothermic reactions that might occur in Hanford Site underground waste storage tanks. These tanks contain many different oxidizable compounds covering a wide range of concentrations. The chemical hazards are a function of several interrelated factors, including the amount of energy (heat) produced, how fast it is produced, and the thermal absorption and heat transfer properties of the system. The reaction path(s) will determine the amount of energy produced and kinetics will determine the rate that it is produced. The tanks also contain many inorganic compounds inert to oxidation. These compounds act as diluents and can inhibit exothermic reactions because of their heat capacity and thus, in contrast to the oxidizable compounds, provide mitigation of hazardous reactions. In this report the energy that may be released when various organic and inorganic compounds react is computed as a function of the reaction-mix composition and the temperature. The enthalpy, or integrated heat capacity, of these compounds and various reaction products is presented as a function of temperature; the enthalpy of a given mixture can then be equated to the energy release from various reactions to predict the maximum temperature which may be reached. This is estimated for several different compositions. Alternatively, the amounts of various diluents required to prevent the temperature from reaching a critical value can be estimated. Reactions taking different paths, forming different products such as N{sub 2}O in place of N{sub 2} are also considered, as are reactions where an excess of caustic is present. Oxidants other than nitrate and nitrite are considered briefly.

  5. Licensing review process of the European Spallation Source (ESS) research facility

    International Nuclear Information System (INIS)

    Brewitz, Erica

    2014-01-01

    On 3 January 2012 a license application under the Radiation Protection Act (SFS, 1988b) for the European Spallation Source research facility was submitted to the Swedish Radiation Safety Authority. The European Spallation Source research facility will be the site of a new and quite unusual kind of neutron source, based on a large proton accelerator that bombards a heavy material with protons. The Swedish Radiation Safety Authority is now reviewing the application. (authors)

  6. Role of compound nuclei in intermediate-energy heavy-ion reactions

    International Nuclear Information System (INIS)

    Moretto, L.G.; Wozniak, G.J.

    1988-05-01

    Hot compound nuclei are frequently produced in intermediate-energy reactions through a variety of processes. Their decay is shown to be an important and at times dominant source of complex fragments, high energy-gamma rays, and even pions

  7. (p,n) reaction at intermediate energy

    International Nuclear Information System (INIS)

    Goodman, C.D.

    1979-01-01

    The use of the (p,n) reaction in exploring effective interactions is reviewed. Some recent data on self-conjugate nuclei taken at the Indiana University Cyclotron Facility (IUCF) are presented, and the differences between low- and high-energy data are emphasized. Experimental problems and techniques used are briefly described. It is concluded that forward-angle (p,n) spectra at energies greater than 100 MeV are dominated by Gamow-Teller (GT) transitions, while Fermi transitions (IAS transitions) dominate near 45 MeV. Prominent GT transitions are expected from a pion-exchange interaction, and it is expected that OPEP is the dominant component of the interaction in the energy range of 100 to 200 MeV. 27 figures, 2 tables

  8. High accuracy measurement of the $^{235}$U(n,f) reaction cross-section in the 10-30 keV neutron energy range

    CERN Multimedia

    The analysis of the neutron flux of n_TOF (in EAR1) revealed an anomaly in the 10-30 keV neutron energy range. While the flux extracted on the basis of the $^{6}$Li(n,t)$^{4}$He and $^{10}$B(n,$\\alpha$)$^{7}$Li reactions mostly agreed with each other and with the results of FLUKA simulations of the neutron beam, the one based on the $^{235}$U(n,f) reaction was found to be systematically lower, independently of the detection system used. A possible explanation is that the $^{235}$U(n,f) crosssection in that energy region, where in principle should be known with an uncertainty of 1%, may be systematically overestimated. Such a finding, which has a negligible influence on thermal reactors, would be important for future fast critical or subcritical reactors. Furthermore, its interest is more general, since the $^{235}$U(n,f) reaction is often used at that energy to determine the neutron flux, or as reference in measurements of fission cross section of other actinides. We propose to perform a high-accuracy, high-r...

  9. Design and verification experiments for the windowless spallation target of the ADS prototype Myrrha

    International Nuclear Information System (INIS)

    Kantrien Van, Tichelen; Kupschus, P.; Arien, B.; Ait Abderrahim, H.

    2003-01-01

    SCKxCEN, the Belgian Nuclear Research Centre, works on the conceptual design and basic engineering of a multipurpose ADS for R and D, dubbed MYRRHA, a small high-performance irradiation facility with fast neutron fluxes up to 1.10 15 n/cm 2 /s to start operation in about 2010. Specific to the MYRRHA ADS system is the choice for a windowless spallation target at the centre of the subcritical core. Apart from the space limitations and material property short-comings, the current and power density figures would make the design of a solid window for the spallation source next to impossible: the chosen 5 mA at the relative low energy of 350 MeV leads to a current density of order 150 μA/cm 2 (as far as we know at least a factor of 3 higher than any window design that has been attempted to meet). This is the main reason for adopting the windowless design for MYRRHA which has as a consequence that the free surface ultimately has to be compatible with the vacuum requirements of the beam transport system of the accelerator. The total beam energy will be dumped into a volume of ca 0.5 1 leading to a heating power density of ca 3 kW/cm 3 . In order to remove this heat from the LM with an average temperature increase of 100 deg C on top of the temperature of the inlet flow of 240 deg C a total flow rate of 101/s at an average flow speed of 2.5 m/s is required. It is suggested from estimates that the evaporation from 'hot spots' with elevated temperatures beyond the average 340 deg C - close to the free surface in the re-circulation zone - is then still acceptable. The design investigations are therefore directed to assess and minimise the re-circulation zone inherent in the free surface formation under the geometry and flow requirements. This paper will summarize the design programme for the windowless design of the spallation source at the centre of the subcritical core. It will include the main findings reported in (Van Tichelen, 2000) and (Van Tichelen, 2001) and the

  10. Mercury flow experiments. 4th report Measurements of erosion rate caused by mercury flow

    CERN Document Server

    Kinoshita, H; Hino, R; Kaminaga, M

    2002-01-01

    The Japan Atomic Energy Research Institute (JAERI) and the High Energy Accelerator Research Organization (KEK) are promoting a construction plan of the Material-Life Science Facility, which is consisted of a Muon Science Facility and a Neutron Scattering Facility, in order to open up the new science fields. The Neutron Scattering Facility will be utilized for advanced fields of Material and Life science using high intensity neutron generated by the spallation reaction of a 1 MW pulsed proton beam and mercury target. Design of the spallation mercury target system aims to obtain high neutron performance with high reliability and safety. Since the target system is using mercury as the target material and contains large amount of radioactive spallation products, it is necessary to estimate reliability for strength of instruments in a mercury flow system during lifetime of the facility. Piping and components in the mercury flow system would be damaged by erosion with mercury flow, since these components will be we...

  11. RF H-minus ion source development in China spallation neutron source

    Science.gov (United States)

    Chen, W.; Ouyang, H.; Xiao, Y.; Liu, S.; Lü, Y.; Cao, X.; Huang, T.; Xue, K.

    2017-08-01

    China Spallation Neutron Source (CSNS) phase-I project currently uses a Penning surface plasma H- ion source, which has a life time of several weeks with occasional sparks between high voltage electrodes. To extend the life time of the ion source and prepare for the CSNS phase-II, we are trying to develop a RF negative hydrogen ion source with external antenna. The configuration of the source is similar to the DESY external antenna ion source and SNS ion source. However several changes are made to improve the stability and the life time. Firstly, Si3N4 ceramic with high thermal shock resistance, and high thermal conductivity is used for plasma chamber, which can endure an average power of 2000W. Secondly, the water-cooled antenna is brazed on the chamber to improve the energy efficiency. Thirdly, cesium is injected directly to the plasma chamber if necessary, to simplify the design of the converter and the extraction. Area of stainless steel exposed to plasma is minimized to reduce the sputtering and degassing. Instead Mo, Ta, and Pt coated materials are used to face the plasma, which makes the self-cleaning of the source possible.

  12. Mitigation and Prediction of Spallation of Oxide Scales on Ferritic Stainless Steel

    Energy Technology Data Exchange (ETDEWEB)

    Chou, Y. S. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Stephens, Elizabeth V. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Xu, Zhijie [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Xu, Wei [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Koeppel, Brian J. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Stevenson, Jeffry W. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)

    2015-02-04

    This report summarizes results from experimental and modeling studies performed by researchers at Pacific Northwest National Laboratory on behalf of the Solid-State Energy Conversion Alliance (SECA) Core Technology Program. The results indicate that application of physical surface modifications, such as surface blasting, prior to application of protective surface coatings can substantially increase oxide scale spallation resistance during long-term exposure to elevated temperatures (e.g., 800-850ºC). To better understand and predict the benefits of surface modification, an integrated modeling framework was developed and applied to the obtained experimental results.

  13. Resonant Electromagnetic Interaction in Low Energy Nuclear Reactions

    Science.gov (United States)

    Chubb, Scott

    2008-03-01

    Basic ideas about how resonant electromagnetic interaction (EMI) can take place in finite solids are reviewed. These ideas not only provide a basis for conventional, electron energy band theory (which explains charge and heat transport in solids), but they also explain how through finite size effects, it is possible to create many of the kinds of effects envisioned by Giuliano Preparata. The underlying formalism predicts that the orientation of the external fields in the SPAWAR protocolootnotetextKrivit, Steven B., New Energy Times, 2007, issue 21, item 10. http://newenergytimes.com/news/2007/NET21.htm^,ootnotetextSzpak, S.; Mosier-Boss, P.A.; Gordon, F.E. Further evidence of nuclear reactions in the Pd lattice: emission of charged particles. Naturwissenschaften 94,511(2007)..has direct bearing on the emission of high-energy particles. Resonant EMI also implies that nano-scale solids, of a particular size, provide an optimal environment for initiating Low Energy Nuclear Reactions (LENR) in the PdD system.

  14. Fast accelerator driven subcritical system for energy production: nuclear fuel evolution

    International Nuclear Information System (INIS)

    Barros, Graiciany de P.; Pereira, Claubia; Veloso, Maria A.F.; Costa, Antonella L.

    2011-01-01

    Accelerators Driven Systems (ADS) are an innovative type of nuclear system, which is useful for long-lived fission product transmutation and fuel regeneration. The ADS consist of a coupling of a sub-critical nuclear core reactor and a proton beam produced by a particle accelerator. These particles are injected into a target for the neutrons production by spallation reactions. The neutrons are then used to maintain the fission chain in the sub-critical core. The aim of this study is to investigate the nuclear fuel evolution of a lead cooled accelerator driven system used for energy production. The fuel studied is a mixture based upon "2"3"2Th and "2"3"3U. Since thorium is an abundant fertile material, there is hope for the thorium-cycle fuels for an accelerator driven sub-critical system. The target is a lead spallation target and the core is filled with a hexagonal lattice. High energy neutrons are used to reduce the negative reactivity caused by the presence of protoactinium, since this effect is most pronounced in the thermal range of the neutron spectrum. For that reason, such material is not added moderator to the system. In this work is used the Monte Carlo code MCNPX 2.6.0, that presents the the depletion/ burnup capability. The k_e_f_f evolution, the neutron energy spectrum in the core and the nuclear fuel evolution using ADS source (SDEF) and kcode-mode are evaluated during the burnup. (author)

  15. Proton injection and RF capture in the national spallation neutron source

    International Nuclear Information System (INIS)

    Luccio, A.U.; Beebe-Wang, J.; Maletic, D.

    1997-01-01

    The accelerator system for the 1 to 5 MW National Spallation Neutron Source (NSNS) consists of a linac followed by a 1 GeV proton accumulator ring. Since the ring is a very high current machine, the injection and rf capture of the protons is deeply affected by transverse and longitudinal space charge effects. Results of numerical simulation of the process are presented together with considerations on methods and results of space charge treatment in high intensity proton storage rings

  16. Cosmic ray-induced spallation recoil tracks in meteoritic phosphates: simulation at the CERN synchrocyclotron

    Energy Technology Data Exchange (ETDEWEB)

    Perron, C [Centre National de la Recherche Scientifique (CNRS), 75 - Paris (France). Inst. d` Astrophysique; [Museum National d` Histoire Naturelle, 75 - Paris (France)

    1994-12-31

    Annealed meteoritic phosphate crystals have been irradiated by 600 MeV protons to simulate cosmic ray irradiation in space. Spallation recoil tracks were then revealed, which mimic fission tracks, specially when observed in the SEM. A production yield of 9.3 {+-} 2.2 x 10{sup 8} spallation track per proton has been obtained for merrillite, and a substantially lower value (2.5 per proton) for apatite. A nominal production yield in space of 6 tracks per year has been derived, which may be used for a rough estimate of spallation track densities in chondritic merrillite. (Author).

  17. Overview of the national spallation neutron source with emphasis on the target station

    International Nuclear Information System (INIS)

    Gabriel, T.A.; Barnes, J.N.; Charlton, L.A.

    1997-01-01

    The technologies that are being utilized to design and build a state-of-the-art neutron spallation source, the National Spallation Neutron Source (NSNS), are discussed. Emphasis is given to the technology issues that present the greatest scientific challenges. The present facility configuration, ongoing analysis and the planned hardware research and development program are also described

  18. A compact Ultra-High Vacuum (UHV) compatible instrument for time of flight-energy measurements of slow heavy reaction products

    Energy Technology Data Exchange (ETDEWEB)

    Kuznetsov, A.V.; Veldhuizen, E.J. van; Westerberg, L.; Lyapin, V.G.; Aleklett, K.; Loveland, W.; Bondorf, J.; Jakobsson, B.; Whitlow, H.J.; El Bouanani, M

    2000-10-01

    A compact Ultra-High Vacuum (UHV) compatible instrument for time of flight-energy measurements of slow heavy reaction products from nuclear reactions has been designed and tested at the CELSIUS storage ring in Uppsala. The construction is based on MicroChannel Plate (MCP) time detectors of the electron mirror type and silicon p-i-n diodes, and permits the detectors to be stacked side-by-side to achieve large solid angle coverage. This kind of telescope measures the Time of Flight (ToF) and Energy (E) of the particle from which one can reconstruct mass. The combination of an ultra-thin cluster gas-jet target and thin carbon emitter foils allows one to measure heavy residues down to an energy of {approx}35 keV/nucleon from the interactions of 400 MeV/nucleon {sup 16}O with {sup nat}Xe gas targets.

  19. A compact Ultra High Vacuum (UHV) compatible instrument for time of flight energy measurements of slow heavy reaction products

    International Nuclear Information System (INIS)

    Kuznetsov, A.V.; Loveland, W.; Jakobsson, B.; Whitlow, H.J.; Bouanani, M. El; Univ. of North Texas, Denton, TX

    2000-01-01

    A compact Ultra High Vacuum (UHV) compatible instrument for time of flight energy measurements of slow heavy reaction products from nuclear reactions has been designed and tested at the CELSIUS storage ring in Uppsala. The construction is based on MicroChannel Plate time detectors of the electron mirror type and silicon p-i-n diodes, and permits the detectors to be stacked side-by-side to achieve large solid angle coverage. This kind of telescope measures the Time of Flight (ToF) and Energy (E) of the particle from which one can reconstruct mass. The combination of an ultra-thin cluster gas-jet target and thin carbon emitter foils allows one to measure heavy residues down to an energy of ∼ 35 keV/nucleon from the interactions of 400 MeV/nucleon 16 O with nat Xe gas targets

  20. A compact Ultra High Vacuum (UHV) compatible instrument for time of flight energy measurements of slow heavy reaction products

    Energy Technology Data Exchange (ETDEWEB)

    Kuznetsov, A.V. [V.G.Khlopin Radium Institute, St. Petersburg (Russian Federation); Uppsala Univ. (Sweden). The Svedberg Lab.; Veldhuizen, E.J. van; Aleklett, K. [Uppsala Univ., (Sweden). Dept. of Radiation Sciences; Westerberg, L. [Uppsala University (Sweden). The Svedberg Lab.; Lyapin, V.G. [V.G.Khlopin Radium Institute, St. Petersburg (Russian Federation); Loveland, W. [Oregon State Univ., Corvallis, OR (United States). Dept. of Chemistry; Bondorf, J. [Niels Bohr Inst., Copenhagen (Denmark); Jakobsson, B. [Lund Univ. (Sweden). Dept. of Physics; Whitlow, H.J. [Lund Univ. (Sweden). Dept. of Nuclear Physics; Bouanani, M. El [Lund Univ. (Sweden). Dept. of Nuclear Physics; Univ. of North Texas, Denton, TX (United States). Dept. of Physics

    2000-07-01

    A compact Ultra High Vacuum (UHV) compatible instrument for time of flight energy measurements of slow heavy reaction products from nuclear reactions has been designed and tested at the CELSIUS storage ring in Uppsala. The construction is based on MicroChannel Plate time detectors of the electron mirror type and silicon p-i-n diodes, and permits the detectors to be stacked side-by-side to achieve large solid angle coverage. This kind of telescope measures the Time of Flight (ToF) and Energy (E) of the particle from which one can reconstruct mass. The combination of an ultra-thin cluster gas-jet target and thin carbon emitter foils allows one to measure heavy residues down to an energy of {approx} 35 keV/nucleon from the interactions of 400 MeV/nucleon {sup 16}O with {sup nat} Xe gas targets.

  1. A compact Ultra-High Vacuum (UHV) compatible instrument for time of flight-energy measurements of slow heavy reaction products

    International Nuclear Information System (INIS)

    Kuznetsov, A.V.; Veldhuizen, E.J. van; Westerberg, L.; Lyapin, V.G.; Aleklett, K.; Loveland, W.; Bondorf, J.; Jakobsson, B.; Whitlow, H.J.; El Bouanani, M.

    2000-01-01

    A compact Ultra-High Vacuum (UHV) compatible instrument for time of flight-energy measurements of slow heavy reaction products from nuclear reactions has been designed and tested at the CELSIUS storage ring in Uppsala. The construction is based on MicroChannel Plate (MCP) time detectors of the electron mirror type and silicon p-i-n diodes, and permits the detectors to be stacked side-by-side to achieve large solid angle coverage. This kind of telescope measures the Time of Flight (ToF) and Energy (E) of the particle from which one can reconstruct mass. The combination of an ultra-thin cluster gas-jet target and thin carbon emitter foils allows one to measure heavy residues down to an energy of ∼35 keV/nucleon from the interactions of 400 MeV/nucleon 16 O with nat Xe gas targets

  2. QMD and JAM calculations for high energy nucleon-nucleus collisions

    International Nuclear Information System (INIS)

    Niita, Koji

    2002-01-01

    We describe the two simulation codes, QMD and JAM (Jet AA Microscopic Transport Model), for high energy nuclear reactions. QMD can treat the nucleus-nucleus reactions as well as nucleon-nucleus reactions based on the molecular dynamics. We have applied the QMD code intensively to nucleon-nucleus reactions and checked its validity. The cross sections obtained by the QMD are now used for evaluation of high energy nuclear data in JAERI. JAM is a hadronic cascade code including the resonance and string model for the hadron-hadron collisions at high energy up to 200 GeV. We have developed a high energy particle transport code NMTC/JAM by including the JAM code for the intra-nuclear cascade part. (author)

  3. Design specification for the European Spallation Source neutron generating target element

    International Nuclear Information System (INIS)

    Aguilar, A.; Sordo, F.; Mora, T.; Mena, L.; Mancisidor, M.; Aguilar, J.; Bakedano, G.; Herranz, I.; Luna, P.; Magan, M.; Vivanco, R.; Jimenez-Villacorta, F.; Sjogreen, K.; Oden, U.; Perlado, J.M.

    2017-01-01

    The paper addresses some of the most relevant issues concerning the thermal hydraulics and radiation damage of the neutron generation target to be built at the European Spallation Source as recently approved after a critical design review. The target unit consists of a set of Tungsten blocks placed inside a wheel of 2.5 m diameter which rotates at some 0.5 Hz in order to distribute the heat generated from incoming protons which reach the target in the radial direction. The spallation material elements are composed of an array of Tungsten pieces which rest on a rotating steel support (the cassette) and are distributed in a cross-flow configuration. The thermal, mechanical and radiation effects resulting from the impact of a 2 GeV proton pulse are analysed in detail as well as an evaluation of the inventory of spallation products. The current design is found to conform to specifications and found to be robust enough to deal with several accident scenarios.

  4. Design specification for the European Spallation Source neutron generating target element

    Energy Technology Data Exchange (ETDEWEB)

    Aguilar, A. [Consorcio ESS-BILBAO. Parque Tecnológico Bizkaia. Poligono Ugaldeguren III, Pol. A, 7B, 48170 Zamudio (Spain); Sordo, F., E-mail: fernando.sordo@essbilbao.org [Consorcio ESS-BILBAO. Parque Tecnológico Bizkaia. Poligono Ugaldeguren III, Pol. A, 7B, 48170 Zamudio (Spain); Instituto de Fusión Nuclear, José Gutiérrez Abascal, 2, 28006 Madrid (Spain); Mora, T. [Consorcio ESS-BILBAO. Parque Tecnológico Bizkaia. Poligono Ugaldeguren III, Pol. A, 7B, 48170 Zamudio (Spain); Mena, L. [Consorcio ESS-BILBAO. Parque Tecnológico Bizkaia. Poligono Ugaldeguren III, Pol. A, 7B, 48170 Zamudio (Spain); Instituto de Fusión Nuclear, José Gutiérrez Abascal, 2, 28006 Madrid (Spain); Mancisidor, M.; Aguilar, J.; Bakedano, G.; Herranz, I.; Luna, P. [Consorcio ESS-BILBAO. Parque Tecnológico Bizkaia. Poligono Ugaldeguren III, Pol. A, 7B, 48170 Zamudio (Spain); Magan, M.; Vivanco, R. [Consorcio ESS-BILBAO. Parque Tecnológico Bizkaia. Poligono Ugaldeguren III, Pol. A, 7B, 48170 Zamudio (Spain); Instituto de Fusión Nuclear, José Gutiérrez Abascal, 2, 28006 Madrid (Spain); Jimenez-Villacorta, F. [Consorcio ESS-BILBAO. Parque Tecnológico Bizkaia. Poligono Ugaldeguren III, Pol. A, 7B, 48170 Zamudio (Spain); Sjogreen, K.; Oden, U. [European Spallation Source ERIC, P.O Box 176, SE-221 00 Lund (Sweden); Perlado, J.M. [Instituto de Fusión Nuclear, José Gutiérrez Abascal, 2, 28006 Madrid (Spain); and others

    2017-06-01

    The paper addresses some of the most relevant issues concerning the thermal hydraulics and radiation damage of the neutron generation target to be built at the European Spallation Source as recently approved after a critical design review. The target unit consists of a set of Tungsten blocks placed inside a wheel of 2.5 m diameter which rotates at some 0.5 Hz in order to distribute the heat generated from incoming protons which reach the target in the radial direction. The spallation material elements are composed of an array of Tungsten pieces which rest on a rotating steel support (the cassette) and are distributed in a cross-flow configuration. The thermal, mechanical and radiation effects resulting from the impact of a 2 GeV proton pulse are analysed in detail as well as an evaluation of the inventory of spallation products. The current design is found to conform to specifications and found to be robust enough to deal with several accident scenarios.

  5. Additional measurements of the radiation environment at the Los Alamos Spallation Radiation Effects Facility at LAMPF

    International Nuclear Information System (INIS)

    Davidson, D.R.; Reedy, R.C.; Greenwood, L.R.; Sommer, W.F.; Wechsler, M.S.

    1987-01-01

    Foil activation dosimetry experiments were conducted in a ''rabbit'' system at the completed Los Alamos Spallation Effects Facility(LASREF). The ''rabbit'' system contains four test tubes spaced radially outward 0.12, 0.18, 0.27, and 0.38 m off beam centerline. Foils were irradiated for 3 to 62 h to measure the neutron flux and energy spectrum radially from beam centerline, along the beamline, and the effect of isotope production (IP) target loadings on the neutron flux in the neutron irradiation locations. Irradiations showed a decrease in the radial flux by a factor of 6 in 0.15 m of iron outside the IP targets. An enhancement was seen in the 24-keV energy region outside 0.15m. There was little difference in the shape of the spectra outside the IP targets and the beam stop with the exception of the high energy tail (energies above 20 MeV). The decrease in the high energy tail outside the beam stop is due to the degradation of the energy of the proton beam in the IP targets. Irradiations outside the beam stop with zero and eight IP targets gave the same spectral shape with the exception of the high energy tail. The magnitude of the integral flux decreased by a factor of two when eight IP targets were present. Irradiations with five ''rabbits'' stacked on top of each other showed no difference in the integral flux below, on and above beam centerline

  6. Additional measurements of the radiation environment at the Los Alamos Spallation Radiation Effects Facility at LAMPF

    International Nuclear Information System (INIS)

    Davidson, D.R.; Reedy, R.C.; Greenwood, L.R.; Sommer, W.F.; Wechsler, M.S.

    1986-01-01

    Foil activation dosimetry experiments were conducted in a ''rabbit'' system at the completed Los Alamos Spallation Radiation Effects Facility (LASREF). The ''raffit'' system contains four tubes spaced radially outward 0.12, 0.18, 0.27, and 0.38 meters off beam centerline. Foils were irradiated for 3 to 62 hours to measure the neutron flux and energy spectrum radially from beam centerline, along the beamline, and the effect of the Isotope Production (IP) target loadings on the neutron flux in the neutron irradiation locations. Irradiations showed a decrease in the radial flux by a factor of 6 in 0.15 meters of iron outside the IP targets. An enchancement was seen in the 24-keV energy region outside 0.15 meters. There was little difference in the shape of the spectra outside the IP targets and the beam stop with the exception of the high energy tail (energies above 20 MeV). The decrease in the high energy tail outside the beam stop is due to the degradation of the energy of the proton beam in the IP targets. Irradiations outside the beam stop with zero and eight IP targets gave the same spectral shape with the exception of the high energy tail. The magnitude of the integral flux decreased by a factor of 2 when eight IP targets were present. Irradiations with five ''rabbits'' stacked on top of each other showed no difference in the integral flux below, on and above beam centerline

  7. Evaluation of internal and external doses from $^{11}C$ produced in the air in high energy proton accelerator tunnels

    CERN Document Server

    Endo, A; Kanda, Y; Oishi, T; Kondo, K

    2001-01-01

    Air has been irradiated with high energy protons at the 12 GeV proton synchrotron to obtain the following parameters essential for the internal dose evaluation from airborne /sup 11/C produced through nuclear spallation reactions: the abundance of gaseous and particulate /sup 11/C, chemical forms, and particle size distribution. It was found that more than 98% of /sup 11/C is present as gas and the rest is aerosol. The gaseous components were only /sup 11/CO and /sup 11/CO/sub 2/ and their proportions were approximately 80% and 20%, respectively. The particulate /sup 11/C was found to be sulphate and/or nitrate aerosols having a log-normal size distribution; the measurement using a diffusion battery showed a geometric mean radius of 0.035 mu m and a geometric standard deviation of 1.8 at a beam intensity of 6.8*10/sup 11/ proton.pulse /sup -1/ and an irradiation time of 9.6 min. By taking the chemical composition and particle size into account, effective doses both from internal and from external exposures pe...

  8. Studies Performed in Preparation for the Spallation Neutron Source Accumulator Ring Commissioning

    CERN Document Server

    Cousineau, Sarah M; Henderson, Stuart; Holmes, Jeffrey Alan; Plum, Michael

    2005-01-01

    The Spallation Neutron Source accumulator ring will compress 1.5?1014, 1 GeV protons from a 1 ms bunch train to a single 695 ns proton bunch for use in neutron spallation. Due to the high beam power, unprecedented control of beam loss will be required in order to control radiation and allow for hands-on maintenance in most areas of the ring. A number of detailed investigations have been performed to understand the primary sources of beam loss and to predict and mitigate problems associated with radiation hot spots in the ring. The ORBIT particle tracking code is used to perform realistic simulations of the beam accumulation in the ring, including detailed modeling of the injection system, transport through the measured magnet fields including higher order multipoles, and beam loss and collimation. In this paper we present the results of a number of studies performed in preparation for the 2006 commissioning of the accumulator ring.

  9. Computed Potential Energy Surfaces and Minimum Energy Pathways for Chemical Reactions

    Science.gov (United States)

    Walch, Stephen P.; Langhoff, S. R. (Technical Monitor)

    1994-01-01

    Computed potential energy surfaces are often required for computation of such parameters as rate constants as a function of temperature, product branching ratios, and other detailed properties. For some dynamics methods, global potential energy surfaces are required. In this case, it is necessary to obtain the energy at a complete sampling of all the possible arrangements of the nuclei, which are energetically accessible, and then a fitting function must be obtained to interpolate between the computed points. In other cases, characterization of the stationary points and the reaction pathway connecting them is sufficient. These properties may be readily obtained using analytical derivative methods. We have found that computation of the stationary points/reaction pathways using CASSCF/derivative methods, followed by use of the internally contracted CI method to obtain accurate energetics, gives usefull results for a number of chemically important systems. The talk will focus on a number of applications including global potential energy surfaces, H + O2, H + N2, O(3p) + H2, and reaction pathways for complex reactions, including reactions leading to NO and soot formation in hydrocarbon combustion.

  10. Spallation neutron source moderator design

    International Nuclear Information System (INIS)

    Charlton, L.A.; Barnes, J.M.; Gabriel, T.A.; Johnson, J.O.

    1998-01-01

    This paper describes various aspects of the spallation neutron source (SNS) moderator design. Included are the effects of varying the moderator location, interaction effects between moderators, and the impact on neutron output when various reflector materials are used. Also included is a study of the neutron output from composite moderators, where it is found that a combination of liquid H 2 O and liquid H 2 can produce a spectrum very similar to liquid methane (L-CH 4 ). (orig.)

  11. Accumulation of the Hf-178m2 isomeric nuclei through spallation with internediate-energy protons of tantalum and rhenium targets

    Czech Academy of Sciences Publication Activity Database

    Karamian, S. A.; Adam, Jindřich; Filossov, DV.; Henzlová, D.; Henzl, V.; Kalinnikov, V. B.; Lebedev, NA.; Novgorodov, A. F.; Collins, CB.; Popescu, II.; UR, CA.

    2002-01-01

    Roč. 489, 1/3 (2002), s. 448-468 ISSN 0168-9002 R&D Projects: GA AV ČR KSK2067107 Keywords : protons * spallation * target activation * radionuclides * isomers * cross-section * multistep model Subject RIV: BG - Nuclear, Atomic and Molecular Physics, Colliders Impact factor: 1.167, year: 2002

  12. Spallation-based science and technology and associated nuclear data requirements

    International Nuclear Information System (INIS)

    Bowman, C.D.; Lisowski, P.W.; Arthur, E.D.

    1990-01-01

    Rapid advances in accelerator technology in recent years promise average proton beam currents as high as 250 mA with energies greater than one GeV. Such an accelerator could produce very high intensities of neutrons and other nuclear particles thus opening up new areas of science and technology. An example is the efficient burning of transuranic and fission product waste. With such a spallation-burner it appears that high-level waste might be converted to low-level waste on a time scale comparable to the human lifespan at a reasonable additional cost for electric power generation. The emphasis of this paper is on the design of a high power proton target for neutron production, on the nuclear data needed to operate this target safely and effectively, and on data requirements for transmutation. It is suggested that a pilot facility consisting of a 1.6 GeV accelerator and target operating at 25 ma is the next major step in developing this technology. Bursts of protons near the terawatt level might also be generated using such an accelerator with a proton accumulator ring. Research prospects based on such proton bursts are briefly described. The status of established nuclear data needs and of accelerator-based sources for nuclear data measurements is reviewed. 6 refs., 8 figs., 2 tabs

  13. Energy changes in massive target-nuclei, induced by high-energy hadronic projectiles

    International Nuclear Information System (INIS)

    Strugalski, Z.; Strugalska-Gola, E.

    1997-01-01

    Now it turned out that it is real to estimate by experiments the energy changes in massive target-nuclei, induced by high-energy hadronic projectiles. The subject matter in this work is to present results of the quantitative estimations of the energy changes in intranuclear matter at various stages of hadron-nucleus collision reactions. Appropriate formulas are proposed for the energy balances - as following from the experimentally based mechanism of the hadron-nucleus collision reactions

  14. HEKATE—A novel grazing incidence neutron scattering concept for the European Spallation Source

    Science.gov (United States)

    Glavic, Artur; Stahn, Jochen

    2018-03-01

    Structure and magnetism at surfaces and buried interfaces on the nanoscale can only be accessed by few techniques, one of which is grazing incidence neutron scattering. While the technique has its strongest limitation in a low signal and large background, due to the low scattering probability and need for high resolution, it can be expected that the high intensity of the European Spallation Source in Lund, Sweden, will make many more such studies possible, warranting a dedicated beamline for this technique. We present an instrument concept, Highly Extended K range And Tunable Experiment (HEKATE), for surface scattering that combines the advantages of two Selene neutron guides with unique capabilities of spatially separated distinct wavelength frames. With this combination, it is not only possible to measure large specular reflectometry ranges, even on free liquid surfaces, but also to use two independent incident beams with tunable sizes and resolutions that can be optimized for the specifics of the investigated samples. Further the instrument guide geometry is tuned for reduction of high energy particle background and only uses low to moderate supermirror coatings for high reliability and affordable cost.

  15. HEKATE-A novel grazing incidence neutron scattering concept for the European Spallation Source.

    Science.gov (United States)

    Glavic, Artur; Stahn, Jochen

    2018-03-01

    Structure and magnetism at surfaces and buried interfaces on the nanoscale can only be accessed by few techniques, one of which is grazing incidence neutron scattering. While the technique has its strongest limitation in a low signal and large background, due to the low scattering probability and need for high resolution, it can be expected that the high intensity of the European Spallation Source in Lund, Sweden, will make many more such studies possible, warranting a dedicated beamline for this technique. We present an instrument concept, Highly Extended K range And Tunable Experiment (HEKATE), for surface scattering that combines the advantages of two Selene neutron guides with unique capabilities of spatially separated distinct wavelength frames. With this combination, it is not only possible to measure large specular reflectometry ranges, even on free liquid surfaces, but also to use two independent incident beams with tunable sizes and resolutions that can be optimized for the specifics of the investigated samples. Further the instrument guide geometry is tuned for reduction of high energy particle background and only uses low to moderate supermirror coatings for high reliability and affordable cost.

  16. Efficient Solar Energy Harvesting and Storage through a Robust Photocatalyst Driving Reversible Redox Reactions.

    Science.gov (United States)

    Zhou, Yangen; Zhang, Shun; Ding, Yu; Zhang, Leyuan; Zhang, Changkun; Zhang, Xiaohong; Zhao, Yu; Yu, Guihua

    2018-06-14

    Simultaneous solar energy conversion and storage is receiving increasing interest for better utilization of the abundant yet intermittently available sunlight. Photoelectrodes driving nonspontaneous reversible redox reactions in solar-powered redox cells (SPRCs), which can deliver energy via the corresponding reverse reactions, present a cost-effective and promising approach for direct solar energy harvesting and storage. However, the lack of photoelectrodes having both high conversion efficiency and high durability becomes a bottleneck that hampers practical applications of SPRCs. Here, it is shown that a WO 3 -decorated BiVO 4 photoanode, without the need of extra electrocatalysts, can enable a single-photocatalyst-driven SPRC with a solar-to-output energy conversion efficiency as high as 1.25%. This SPRC presents stable performance over 20 solar energy storage/delivery cycles. The high efficiency and stability are attributed to the rapid redox reactions, the well-matched energy level, and the efficient light harvesting and charge separation of the prepared BiVO 4 . This demonstrated device system represents a potential alternative toward the development of low-cost, durable, and easy-to-implement solar energy technologies. © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  17. Optimal Electrical Energy Slewing for Reaction Wheel Spacecraft

    Science.gov (United States)

    Marsh, Harleigh Christian

    The results contained in this dissertation contribute to a deeper level of understanding to the energy required to slew a spacecraft using reaction wheels. This work addresses the fundamental manner in which spacecrafts are slewed (eigenaxis maneuvering), and demonstrates that this conventional maneuver can be dramatically improved upon in regards to reduction of energy, dissipative losses, as well as peak power. Energy is a fundamental resource that effects every asset, system, and subsystem upon a spacecraft, from the attitude control system which orients the spacecraft, to the communication subsystem to link with ground stations, to the payloads which collect scientific data. For a reaction wheel spacecraft, the attitude control system is a particularly heavy load on the power and energy resources on a spacecraft. The central focus of this dissertation is reducing the burden which the attitude control system places upon the spacecraft in regards to electrical energy, which is shown in this dissertation to be a challenging problem to computationally solve and analyze. Reducing power and energy demands can have a multitude of benefits, spanning from the initial design phase, to in-flight operations, to potentially extending the mission life of the spacecraft. This goal is approached from a practical standpoint apropos to an industry-flight setting. Metrics to measure electrical energy and power are developed which are in-line with the cost associated to operating reaction wheel based attitude control systems. These metrics are incorporated into multiple families of practical high-dimensional constrained nonlinear optimal control problems to reduce the electrical energy, as well as the instantaneous power burdens imposed by the attitude control system upon the spacecraft. Minimizing electrical energy is shown to be a problem in L1 optimal control which is nonsmooth in regards to state variables as well as the control. To overcome the challenge of nonsmoothness, a

  18. [Studies of target fragmentation in intermediate energy, relativistic and ultra-relativistic nuclear collisions

    International Nuclear Information System (INIS)

    Loveland, W.D.

    1991-08-01

    The work described herein is part of a project involving the study of low energy ( 250 MeV/A) heavy ion reactions. In the low energy regime, we published a monograph on the properties of the heaviest elements and used that publication as a basis for making a set of ''best'' semi-empirical predictions of heavy element decay properties. The intermediate energy research effort focussed upon the completion of studies already begun and the initiation of a number of new experiments. In our study of a interaction of 21 MeV/nucleon 129 Xe with 197 Au, we compared the characteristics of the observed deep inelastic phenomena with various models of dissipative reactions and found significant discrepancies between observations and predictions. These discrepancies seemed to be caused by an improper treatment of pre-equilibrium in the early stages of the collision. In our study of the relativistic interaction of 400 MeV/nucleon 12 C with 197 Au, we reported the first direct physical measurement of the properties of the spallation residues from a nucleus-nucleus collision. We found the residue energies to be much lower than those predicted by the intranuclear cascade model, indicating some substantial modifications of that model are needed. But, we also found, indications of significant, non-zero values of the residue transverse momentum, a finding that calls into question the interpretation of a number of radiochemical recoil studies of the kinematics of high energy reactions. A program of performing numerical simulations of intermediate and high energy nuclear collisions using the QMD model was initiated

  19. Big-bang nucleosynthesis with a long-lived CHAMP including He4 spallation process

    Science.gov (United States)

    Yamanaka, Masato; Jittoh, Toshifumi; Kohri, Kazunori; Koike, Masafumi; Sato, Joe; Sugai, Kenichi; Yazaki, Koichi

    2014-03-01

    We propose helium-4 spallation processes induced by long-lived stau in supersymmetric standard models, and investigate an impact of the processes on light elements abundances. We show that, as long as the phase space of helium-4 spallation processes is open, they are more important than stau-catalyzed fusion and hence constrain the stau property. This talk is based on the work of ref. [1].

  20. Commissioning of the Superconducting Linac at the Spallation Neutron Source (SNS)

    International Nuclear Information System (INIS)

    Kim, Sang-Ho; Campisi, Isidoro E.

    2007-01-01

    The use of superconducting radiofrequency (SRF) cavities in particle accelerator is becoming more widespread. Among the projects that make use of that technology is the Spallation Neutron Source, where H-ions are accelerated to about 1 GeV, mostly making use of niobium elliptical cavities. SNS will use the accelerated short (about 700 ns) sub-bunches of protons to generate neutrons by spallation, which will in turn allow probing structural and magnetic properties of new and existing materials. The SNS superconducting linac is the largest application of RF superconductivity to come on-line in the last decade. The SRF cavities, operated at 805 MHz, were designed, built and integrated into cryomodules at Jefferson Lab and installed and tested at SNS. SNS is also the first proton-like accelerator which uses SRF cavities in a pulse mode. Many of the details of the cavity performance are peculiar to this mode of operation, which is also being applied to lepton accelerators (TESLA test facility and X-FEL at DESY and the international linear collider project). Thanks to the low frequency of the SNS superconducting cavities, operation at 4.2 K has been possible without beam energy degradation, even though the cavities and cryogenic systems were originally designed for 2.1 K operation. The testing of the superconducting cavities, the operating experience with beam and the performance of the superconducting linac will be presented

  1. Spallation neutrons pulsed sources

    International Nuclear Information System (INIS)

    Carpenter, J.

    1996-01-01

    This article describes the range of scientific applications which can use these pulsed neutrons sources: Studies on super fluids, measures to verify the crawling model for the polymers diffusion; these sources are also useful to study the neutron disintegration, the ultra cold neutrons. In certain applications which were not accessible by neutrons diffusion, for example, radiations damages, radionuclides production and activation analysis, the spallation sources find their use and their improvement will bring new possibilities. Among others contributions, one must notice the place at disposal of pulsed muons sources and neutrinos sources. (N.C.). 3 figs

  2. Spallation nucleosynthesis by accelerated charged-particles

    International Nuclear Information System (INIS)

    Goriely, S.

    2008-01-01

    Recent observations have suggested the presence of radioactive elements, such as Pm and 84≤Z≤99 elements) at the surface of the magnetic star HD101065, also known as Przybylski's star. This star is know to be a chemically peculiar star and its anomalous 38 30 heavy elements can be achieved. In this nucleosynthesis process, the secondary-neutron captures play a crucial role. The most attractive feature of the spallation process is the systematic production of Pm and Tc and the possible synthesis of actinides and sub-actinides.Based on such a parametric model, it is also shown that intense fluences of accelerated charged-particles interacting with surrounding material can efficiently produce elements heavier than iron. Different regimes are investigated and shown to be at the origin of p- and s-nuclei in the case of high-fluence low-flux events and r-nuclei for high-fluence high-flux irradiations. The possible existence of such irradiation events need to be confirmed by hydrodynamics simulations, but most of all by spectroscopic observations through the detection of short-lived radio-elements

  3. Measurement of isotopic cross sections of the fission fragments produced in 500 AMeV {sup 208}Pb + p reaction; Etude de la production des fragments de fission issus de la reaction {sup 208}Pb + p a 500 AMeV

    Energy Technology Data Exchange (ETDEWEB)

    Fernandez-Dominguez, B

    2003-03-01

    The aim of this work is the study of the fission fragments produced in the spallation reaction {sup 208}Pb + p at 500 AMeV. The fission fragments from Z=23 up to Z=59 have been detected and identified by using the inverse kinematics technique with the high-resolution spectrometer FRS. The production cross sections and the recoil velocities of 430 nuclei have been measured. The measured data have been compared with previous data. The isotopic distributions show a high precision. However, the absolute value of the fission cross section is higher than expected. From the experimental data the characteristics of the average fissioning system have been reconstructed (Z{sub fis}, A{sub fis}, E*{sub fis}). In addition, the number of post-fission neutrons emitted from the fission fragments, v{sub post}, has been determined by using a new method. The experimental data have been compared to the two-steps models describing the spallation reaction. The impact of the model parameters on the observables has been analysed and the reasons Leading to the observed differences between the codes are also presented. This analyse shows a good agreement with the INCL4+ABLA code. (author)

  4. Construction and operation of the Spallation Neutron Source: Draft environmental impact statement. Volume 1

    International Nuclear Information System (INIS)

    1998-12-01

    DOE proposes to construct and operate a state-of-the-art, short-pulsed spallation neutron source comprised of an ion source, a linear accelerator, a proton accumulator ring, and an experiment building containing a liquid mercury target and a suite of neutron scattering instrumentation. The proposed Spallation Neutron Source would be designed to operate at a proton beam power of 1 megawatt. The design would accommodate future upgrades to a peak operating power of 4 megawatts. These upgrades may include construction of a second proton accumulation ring and a second target. The US needs a high-flux, short-pulsed neutron source to provide the scientific and industrial research communities with a much more intense source of pulsed neutrons for neutron scattering research than is currently available, and to assure the availability of a state-of-the-art facility in the decades ahead. This next-generation neutron source would create new scientific and engineering opportunities. In addition, it would help replace the neutron science capacity that will be lost by the eventual shutdown of existing sources as they reach the end of their useful operating lives in the first half of the next century. This document analyzes the potential environmental impacts from the proposed action and the alternatives. The analysis assumes a facility operating at a power of 1 MW and 4 MW over the life of the facility. The two primary alternatives analyzed in this EIS are: the proposed action (to proceed with building the Spallation Neutron Source) and the No-Action Alternative. The No-Action Alternative describes the expected condition of the environment if no action were taken. Four siting alternatives for the Spallation Neutron Source are evaluated: Oak Ridge National Laboratory, Oak Ridge, TN, (preferred alternative); Argonne National Laboratory, Argonne, IL (US); Brookhaven National Laboratory, Upton, NY; and Los Alamos National Laboratory, Los Alamos, NM

  5. Magnets for the national spallation neutron source accumulator ring

    International Nuclear Information System (INIS)

    Tuozzolo, J.; Brodowski, J.; Danby, G.

    1997-01-01

    The National Spallation Neutron Source Accumulator Ring will require large aperture dipole magnets, strong focusing quadrupole magnets, and smaller low field dipole, quadrupole, and sextupole correcting magnets. All of the magnets will provide a fixed magnetic field throughout the accumulator's fill/storage/extraction cycle. Similar fixed field magnets will also be provided for the beam transport systems. Because of the high intensity in the accumulator, the magnets must be designed with high tolerances for optimum field quality and for the high radiation environment which may be present at the injection/extraction areas, near the collimators, and near the target area. Field specifications and field plots are presented as well as planned fabrication methods and procedures, cooling system design, support, and installation

  6. Some safety studies of the MEGAPIE spallation source target performed using computational fluid dynamics

    International Nuclear Information System (INIS)

    Smith, B.L.

    2011-01-01

    Such a target forms part of the evolutionary Accelerator-Driven System (ADS) concept in which neutrons are generated in an otherwise sub-critical core by spallation reactions resulting from bombardment by a proton beam. The international project MEGAPIE had the objective of demonstrating the feasibility of the spallation process for a particular target design under strict test conditions. The test was carried over a period of four months at the end of 2006 at the SINQ facility of the Paul Scherrer Institute in Switzerland. The design studies carried out for the MEGAPIE target prior to irradiation using Computational Fluid Dynamics (CFD) resulted in an optimum flow configuration being defined for the coolant circulation. Simultaneously, stresses in the structural components were examined using Finite Element Method (FEM) techniques. To this purpose, an interface program was written which enabled different specialist groups to carry out the thermal hydraulics and structural mechanics analyses within the project with fully consistent model data. Results for steady-state operation of the target show that the critical lower target components are adequately cooled, and that stresses and displacements are well within tolerances. Transient analyses were also performed to demonstrate the robustness of the design in the event of abnormal operation, including pump failure and burn-through of the target casing by the proton beam. In the latter case, the CFD analyses complemented and extended full-scale tests. (author)

  7. Some safety studies of the MEGAPIE spallation source target performed using computational fluid dynamics

    Energy Technology Data Exchange (ETDEWEB)

    Smith, B.L., E-mail: brian.smith@psi.ch [Paul Scherrer Institute, OHSA/C08, 5232 Villigen PSI (Switzerland)

    2011-07-01

    Such a target forms part of the evolutionary Accelerator-Driven System (ADS) concept in which neutrons are generated in an otherwise sub-critical core by spallation reactions resulting from bombardment by a proton beam. The international project MEGAPIE had the objective of demonstrating the feasibility of the spallation process for a particular target design under strict test conditions. The test was carried over a period of four months at the end of 2006 at the SINQ facility of the Paul Scherrer Institute in Switzerland. The design studies carried out for the MEGAPIE target prior to irradiation using Computational Fluid Dynamics (CFD) resulted in an optimum flow configuration being defined for the coolant circulation. Simultaneously, stresses in the structural components were examined using Finite Element Method (FEM) techniques. To this purpose, an interface program was written which enabled different specialist groups to carry out the thermal hydraulics and structural mechanics analyses within the project with fully consistent model data. Results for steady-state operation of the target show that the critical lower target components are adequately cooled, and that stresses and displacements are well within tolerances. Transient analyses were also performed to demonstrate the robustness of the design in the event of abnormal operation, including pump failure and burn-through of the target casing by the proton beam. In the latter case, the CFD analyses complemented and extended full-scale tests. (author)

  8. Transfer and breakup reactions at intermediate energies

    International Nuclear Information System (INIS)

    Stokstad, R.G.

    1986-04-01

    The origin of the quasi-elastic peak in peripheral heavy-ion reactions is discussed in terms of inelastic scattering and transfer reactions to unbound states of the primary projectile-like fragment. The situation is analogous to the use of reverse kinematics in fusion reactions, a technique in which the object of study is moving with nearly the beam velocity. It appears that several important features of the quasi-elastic peak may be explained by this approach. Projectile-breakup reactions have attractive features for the study of nuclear structure. They may also be used to determine the partition of excitation energy in peripheral reactions. At intermediate energies, neutron-pickup reactions leading to four-body final states become important. Examples of experiments are presented that illustrate these points. 15 refs., 14 figs

  9. Proceedings of the workshop on neutron instrumentation for a long-pulse spallation source

    International Nuclear Information System (INIS)

    Alonso, J.; Schroeder, L.; Pynn, R.

    1995-01-01

    This workshop was carried out under the auspices of the Lawrence Berkeley National Laboratory Pulsed Spallation Source activity and its Pulsed Spallation Source Committee (PSSC). One of our activities has been the sponsorship of workshops related to neutron production by pulsed sources. At the Crystal City PSSC meeting a decision was made to hold a workshop on the instrumentation opportunities at a long-pulse spallation source (LPSS). The enclosed material represents the results of deliberations of the three working groups into which the participants were divided, covering elastic scattering, inelastic scattering and fundamental physics, as well as contributions from individual participants. We hope that the material in this report will be useful to the neutron scattering community as it develops a road-map for future neutron sources. The workshop was held at LBNL in mid-April with about sixty very dedicated participants from the US and abroad. This report presents the charge for the workshop: Based on the bench mark source parameters provided by Gary Russell, determine how a suite of spectrometers in each of the three working group's area of expertise would perform at an LPSS and compare this performance with that of similar spectrometers at a continuous source or a short-pulse source. Identify and discuss modifications to these spectrometers that would enhance their performance at an LPSS. Identify any uncertainties in the analysis of spectrometer performance that require further research. Describe what R ampersand D is needed to resolve these issues. Discuss how the performance of instruments would be affected by changes in source parameters such as repetition rate, proton pulse length, and the characteristic time of pulse tails. Identify beneficial changes that could become goals for target/moderator designers. Identify novel methods that might be applied at an LPSS. Selected papers are indexed separately for inclusion in the Energy Science and Technology

  10. Electron Cloud Mitigation in the Spallation Neutron Source Ring

    International Nuclear Information System (INIS)

    Wei, J.; Blaskiewicz, Michael; Brodowski, J.; Cameron, P.; Davino, Daniele; Fedotov, A.; He, P.; Hseuh, H.; Lee, Y.Y.; Ludewig, H.; Meng, W.; Raparia, D.; Tuozzolo, J.; Zhang, S.Y.; Catalan-Lasheras, N.; Macek, R.J.; Furman, Miguel A.; Aleksandrov, A.; Cousineau, S.; Danilov, V.; Henderson, S.

    2008-01-01

    The Spallation Neutron Source (SNS) accumulator ring is designed to accumulate, via H - injection, protons of 2 MW beam power at 1 GeV kinetic energy at a repetition rate of 60 Hz [1]. At such beam intensity, electron-cloud is expected to be one of the intensity-limiting mechanisms that complicate ring operations. This paper summarizes mitigation strategy adopted in the design, both in suppressing electron-cloud formation and in enhancing Landau damping, including tapered magnetic field and monitoring system for the collection of stripped electrons at injection, TiN coated beam chamber for suppression of the secondary yield, clearing electrodes dedicated for the injection region and parasitic on BPMs around the ring, solenoid windings in the collimation region, and planning of vacuum systems for beam scrubbing upon operation

  11. Electron-cloud mitigation in the spallation neutron source ring

    International Nuclear Information System (INIS)

    Wei, J.; Blaskiewicz, M.; Brodowski, J.; Cameron, P.; Davino, D.; Fedotov, A.; He, P.; Hseuh, H.; Lee, Y.Y.; Meng, W.; Raparia, D.; Tuozzolo, J.; Zhang, S.Y.; Danilov, V.; Henderson, S.; Furman, M.; Pivi, M.; Macek, R.

    2003-01-01

    The Spallation Neutron Source (SNS) accumulator ring is designed to accumulate, via H- injection, protons of 2 MW beam power at 1 GeV kinetic energy at a repetition rate of 60 Hz [1]. At such beam intensity, electron cloud is expected to be one of the intensity-limiting mechanisms that complicate ring operations. This paper summarizes mitigation strategy adopted in the design, both in suppressing electron-cloud formation and in enhancing Landau damping, including tapered magnetic field and monitoring system for the collection of stripped electrons at injection, TiN coated beam chamber for suppression of the secondary yield, clearing electrodes dedicated for the injection region and parasitic on BPMs around the ring, solenoid windings in the collimation region, and planning of vacuum systems for beam scrubbing upon operation

  12. Computing the Free Energy along a Reaction Coordinate Using Rigid Body Dynamics.

    Science.gov (United States)

    Tao, Peng; Sodt, Alexander J; Shao, Yihan; König, Gerhard; Brooks, Bernard R

    2014-10-14

    The calculations of potential of mean force along complex chemical reactions or rare events pathways are of great interest because of their importance for many areas in chemistry, molecular biology, and material science. The major difficulty for free energy calculations comes from the great computational cost for adequate sampling of the system in high-energy regions, especially close to the reaction transition state. Here, we present a method, called FEG-RBD, in which the free energy gradients were obtained from rigid body dynamics simulations. Then the free energy gradients were integrated along a reference reaction pathway to calculate free energy profiles. In a given system, the reaction coordinates defining a subset of atoms (e.g., a solute, or the quantum mechanics (QM) region of a quantum mechanics/molecular mechanics simulation) are selected to form a rigid body during the simulation. The first-order derivatives (gradients) of the free energy with respect to the reaction coordinates are obtained through the integration of constraint forces within the rigid body. Each structure along the reference reaction path is separately subjected to such a rigid body simulation. The individual free energy gradients are integrated along the reference pathway to obtain the free energy profile. Test cases provided demonstrate both the strengths and weaknesses of the FEG-RBD method. The most significant benefit of this method comes from the fast convergence rate of the free energy gradient using rigid-body constraints instead of restraints. A correction to the free energy due to approximate relaxation of the rigid-body constraint is estimated and discussed. A comparison with umbrella sampling using a simple test case revealed the improved sampling efficiency of FEG-RBD by a factor of 4 on average. The enhanced efficiency makes this method effective for calculating the free energy of complex chemical reactions when the reaction coordinate can be unambiguously defined by a

  13. Invited talks (Abstracts only) The spallation neutron source: New ...

    Indian Academy of Sciences (India)

    The spallation neutron source (SNS) facility became operational in the spring of 2006, and is ... torate at ORNL providing the opportunity to develop science and instrumentation pro- ... tion, information technology, biotechnology, and health.

  14. High power operation of the polyphase resonant converter modulator system for the spallation neutron source linear accelerator

    CERN Document Server

    Reass, W A; Baca, D M; Doss, J D; Gonzáles, J M; Gribble, R F; Trujillo, P G

    2003-01-01

    The spallation neutron source (SNS) is a new 1.4 MW average power beam, 1 GeV accelerator being built at Oak Ridge national laboratory. The accelerator requires 15 "long-pulse" converter-modulator stations each providing a maximum of 11 MW pulses with a 1.1 MW average power. Two variants of the converter-modulator are utilized, an 80 kV and a 140 kV design, the voltage dependant on the type of klystron load. The converter-modulator can be described as a resonant zero-voltage- switching polyphase boost inverter. As noted in Figure 1, each converter modulator derives its buss voltage from a standard 13.8 kV to 2100 Y (1.5 MVA) substation cast-core transformer. The substation also contains harmonic traps and filters to accommodate IEEE 519 and 141 regulations. Each substation is followed by an SCR preregulator to accommodate system voltage changes from no load to full load, in addition to providing a soft-start function. Energy storage and filtering is provided by special low inductance self-clearing metallized ...

  15. SUPERCONDUCTING LINAC FOR THE SPALLATION NEUTRON SOURCE

    International Nuclear Information System (INIS)

    STOVALL, J.; NATH, S.

    2000-01-01

    The Spallation Neutron Source (SNS) linac is comprised of both normal and superconducting rf (SRF) accelerating structures. The SRF linac accelerates the beam from 186 to 1250 MeV through 117 elliptical, multi-cell niobium cavities. This paper describes the SRF linac architecture, physics design considerations, cavity commissioning, and the expected beam dynamics performance

  16. High energy collisions of nuclei: experiments

    International Nuclear Information System (INIS)

    Heckman, H.H.

    1977-09-01

    Heavy-ion nuclear reactions with projectile energies up to 2.1 GeV/A are reviewed. The concept of ''rapidity'' is elucidated, and the reactions discussed are divided into sections dealing with target fragmentation, projectile fragmentation, and the intermediate region, with emphasis on the production of light nuclei in high-energy heavy-ion collisions. Target fragmentation experiments using nuclear emulsion and AgCl visual track detectors are also summarized. 18 figures

  17. Observation of gaseous nitric acid production at a high-energy proton accelerator facility

    CERN Document Server

    Kanda, Y; Nakajima, H

    2005-01-01

    High-energy protons and neutrons produce a variety of radionuclides as well as noxious and oxidative gases, such as ozone and nitric acid, in the air mainly through the nuclear spallation of atmospheric elements. Samples were collected from the surfaces of magnets, walls, and floors in the neutrino beamline tunnel and the target station of the KEK 12-GeV proton synchrotron facility by wiping surfaces with filter paper. Considerably good correlations were found between the amounts of nitrate and tritium and between those of nitrate and /sup 7/Be. This finding gives evidence that at high-energy proton facilities, nitric acid is produced in the radiolysis of air in beam- loss regions. Also, the nitric acid on the surfaces was found to be desorbed and tended to be more uniform throughout the tunnel due to air circulation. The magnitude of diminishing from the surfaces was in the order of tritium>nitrate>/sup 7/Be1).

  18. Measurement of isotopic cross sections of the fission fragments produced in 500 AMeV 208Pb + p reaction

    International Nuclear Information System (INIS)

    Fernandez-Dominguez, B.

    2003-03-01

    The aim of this work is the study of the fission fragments produced in the spallation reaction 208 Pb + p at 500 AMeV. The fission fragments from Z=23 up to Z=59 have been detected and identified by using the inverse kinematics technique with the high-resolution spectrometer FRS. The production cross sections and the recoil velocities of 430 nuclei have been measured. The measured data have been compared with previous data. The isotopic distributions show a high precision. However, the absolute value of the fission cross section is higher than expected. From the experimental data the characteristics of the average fissioning system have been reconstructed (Z fis , A fis , E* fis ). In addition, the number of post-fission neutrons emitted from the fission fragments, v post , has been determined by using a new method. The experimental data have been compared to the two-steps models describing the spallation reaction. The impact of the model parameters on the observables has been analysed and the reasons Leading to the observed differences between the codes are also presented. This analyse shows a good agreement with the INCL4+ABLA code. (author)

  19. New findings on the onset of thermal disassembly in spallation reactions; Nouvelles approches pour l'etude de la multifragmentation thermique dans la spallation

    Energy Technology Data Exchange (ETDEWEB)

    Napolitani, P

    2004-09-15

    Thermal multifragmentation is the process of multi body disassembly of a hot nucleus when the excitation is almost purely thermal i.e. dynamical effects like compression (characteristic of ion-ion collisions at Fermi energy) are negligible. Suited reactions are proton induced collision or ion-ion abrasion at relativistic incident energy. Thus we measured four systems at FRS (Fragment separator, GSI, Darmstadt) in inverse kinematics: Fe{sup 56}+p, Fe{sup 56}+Ti(nat), Xe{sup 136}+p, Xe{sup 136}+Ti(nat) a 1 A*GeV. The inverse kinematics allows to observe all particles without any threshold in energy. This is a great advantage compared to experiments in direct kinematics, because only in inverse kinematics it is possible to obtain complete velocity spectra (without a hole for low velocities) for fully identified isotopes. The complex shape of the velocity spectra allows to identify the different deexcitation channels and it clearly shows the transition from a chaotic-dominated process (Gaussian cloud in velocity space) to a direct Coulomb- (or eventually expansion-) dominated process (shell of a sphere in velocity space). Different possible descriptions of the reaction process are discussed, based either on asymmetric fission or multifragmentation. The resulting physical picture is especially interesting for the Fe{sup 56}+p, and Xe{sup 136}+p systems: proton induced collisions could result in the split of the system in two or more fragments due to a fast break-up process. In this case, the configuration of the break-up partition is very asymmetric. The discussion will be extended to other characteristics, like the restoring of nuclear structure features in the isotopic production and the temperature dependence of the isotopic composition of the residues. (author)

  20. Spin distribution in preequilibrium reactions for 48Ti + n.

    Energy Technology Data Exchange (ETDEWEB)

    Dashdorj, Dugersuren [North Carolina State Univ., Raleigh, NC (United States)

    2005-04-12

    Cross section measurements were made of prompt γ-ray production as a function of incident neutron energy on a 48Ti sample. Partial γ-ray cross sections for transitions in 45-48Ti, 44-48Sc, and 42-45Ca have been determined. Energetic neutrons were delivered by the Los Alamos National Laboratory spallation neutron source located at the LANSCE/WNR facility. The prompt-reaction γ rays were detected with the large-scale Compton-suppressed germanium array for neutron induced excitations (GEANIE). Neutron energies were determined by the time-of-flight technique. The γ-ray excitation functions were converted to partial γ-ray cross sections taking into account the dead-time correction, target thickness, detector efficiency and neutron flux (monitored with an in-line fission chamber). The data are presented for neutron energies En between 1 to 200 MeV. These results are compared with model calculations which include compound nuclear and pre-equilibrium emission. The model calculations are performed using the STAPRE reaction code for En up to 20 MeV and the GNASH reaction code for En up to 120 MeV. Using the GNASH reaction code the effect of the spin distribution in preequilibrium reactions has been investigated. The preequilibrium reaction spin distribution was calculated using the quantum mechanical theory of Feshbach, Kerman, and Koonin (FKK). The multistep direct (MSD) part of the FKK theory was calculated for a one-step process. The contribution from higher steps is estimated to be small. The spin distribution of the multistep compound (MSC) part of FKK theory is assumed to be the same as in the compound nucleus. The FKK preequilibrium spin distribution was incorporated into the GNASH calculations and the γ-ray production cross sections were calculated and compared with experimental data. The difference in the partial γ-ray cross sections using spin distributions with and without