Effects of energy variations of ions influencing a target on implantation

International Nuclear Information System (INIS)

Astakhov, V.P.; Rubtsov, V.A.; Aranovich, R.M.; Pavlov, P.V.

1981-01-01

In cases of phosphorus and boron ion implantation into silicon the dependence of electrophysical properties of ion-doped layers and target material near the layer boundaries on energy variation conditions of influencing ions is observed. A physical model explaining the dependence is proposed. It is found that for the target, being at room temperature, after successive annealing the qualitative characteristics of conditions (i.e. energy increase and decrease) on implantation of phosphorus ions into p-silicon and boron ions into n-silicon, as well as the value of energy stages, define rhosub(l) ion-doped layer resistivity and tausub(mc) nonequilibrium minority carrier lifetime in the base of p-n transitions. The essence of the effects observed is that for equal sets of Esub(i) ion energy values and PHIsub(i) corresponding phases at maximum energy used exceeding 30 keV, successive energy increase during implantation, when E 1 2 1 mode), leads to smaller rhosub(e) values and greater tausub(mc) than in case of successive energy decrease, when E 1 >E 2 >...E(E 2 mode) for any fixed annealing temperature. In cases when the maximum energy does not exceed 30 KeV, the E 1 and E 2 modes lead to analogous rhosub(e) and tausub(mc) values. The E 2 mode leads to enrichment of the ion-implanted layer with associations and complexes on the basis of interstitial atoms in comparison with the E 1 mode. The associations and complexes on thermal treatment are reformed into the higher-temperature interstitial complexes increasing rhosub(e) and decreasing tausub(mc). Supposition about the effect of these complexes and processes of structural transformations on annealing, hampering-improvement of structural properties of the ion-implanted layer and a crystal region bordered on it [ru

Red Phosphorus-Embedded Cross-Link-Structural Carbon Films as Flexible Anodes for Highly Reversible Li-Ion Storage

Energy Technology Data Exchange (ETDEWEB)

Ruan, Jiafeng [School of Materials; Yuan, Tao [School of Materials; Pang, Yuepeng [School of Materials; Xu, Xinbo [School of Materials; Yang, Junhe [School of Materials; Hu, Wenbin; Zhong, Cheng; Ma, Zi-Feng [Shanghai Electrochemical Energy Devices Research Center,; Bi, Xuanxuan [Chemical; Zheng, Shiyou [School of Materials

2017-10-06

Red phosphorus (P) is considered to be one of the most attractive anodic materials for lithium-ion batteries (LIBs) due to its high theoretical capacity of 2596 mAh g–1. However, intrinsic characteristics such as the poor electronic conductivity and large volume expansion at lithiation impede the development of red P. Here, we design a new strategy to embed red P particles into a cross-link-structural carbon film (P–C film), in order to improve the electronic conductivity and accommodate the volume expansion. The red P/carbon film is synthesized via vapor phase polymerization (VPP) followed by the pyrolysis process, working as a flexible binder-free anode for LIBs. High cycle stability and good rate capability are achieved by the P–C film anode. With 21% P content in the film, it displays a capacity of 903 mAh g–1 after 640 cycles at a current density of 100 mA g–1 and a capacity of 460 mAh g–1 after 1000 cycles at 2.0 A g–1. Additionally, the Coulombic efficiency reaches almost 100% for each cycle. The superior properties of the P–C films together with their facile fabrication make this material attractive for further flexible and high energy density LIB applications.

Surface studies with high-energy ion beams

Energy Technology Data Exchange (ETDEWEB)

Stensgaard, Ivan [Aarhus Univ. (Denmark). Inst. of Physics

1992-07-01

High-energy ion scattering is an extremely useful technique for surface studies. Three methods for surface composition analysis (Rutherford backscattering, nuclear-reaction analysis and elastic recoil detection) are discussed. Directional effects in ion-beam surface interactions (shadowing and blocking) form the basis for surface structure analysis with high-energy ion beams and these phenomena are addressed in some detail. It is shown how surface relaxation and reconstruction, as well as positions of adsorbed atoms, can be determined by comparison with computer simulations. A special technique called transmission channelling is introduced and shown to be particularly well suited for studies of adsorption positions, even of hydrogen. Recent developments in the field are demonstrated by discussing a large number of important (experimental) applications which also include surface dynamics and melting, as well as epitaxy and interface structure. (author).

High-energy ion tail formation due to ion acoustic turbulence in the TRIAM-1 tokamak

Energy Technology Data Exchange (ETDEWEB)

Nakamura, Kazuo; Hiraki, Naoji; Nakamura, Yukio; Itoh, Satoshi [Kyushu Univ., Fukuoka (Japan). Research Inst. for Applied Mechanics

1982-02-01

The two-component ion energy spectra observed in the TRIAM-1 tokamak are explained as a result of the high-energy ion tail formation due to ion acoustic turbulence driven by a toroidal current pulse for turbulent heating.

Generation of intense, high-energy ion pulses by magnetic compression of ion rings

International Nuclear Information System (INIS)

Kapetanakos, C.A.

1981-01-01

A system based on the magnetic compression of ion rings, for generating intense (High-current), high-energy ion pulses that are guided to a target without a metallic wall or an applied external magnetic field includes a vacuum chamber; an inverse reflex tetrode for producing a hollow ion beam within the chamber; magnetic coils for producing a magnetic field, bo, along the axis of the chamber; a disc that sharpens a magnetic cusp for providing a rotational velocity to the beam and causing the beam to rotate; first and second gate coils for producing fast-rising magnetic field gates, the gates being spaced apart, each gate modifying a corresponding magnetic mirror peak (Near and far peaks) for trapping or extracting the ions from the magnetic mirror, the ions forming a ring or layer having rotational energy; a metal liner for generating by magnetic flux compression a high, time-varying magnetic field, the time-varying magnetic field progressively increasing the kinetic energy of the ions, the magnetic field from the second gate coil decreasing the far mirror peak at the end of the compression for extracting the trapped rotating ions from the confining mirror; and a disc that sharpens a magnetic half-cusp for increasing the translational velocity of the ion beam. The system utilizes the self-magnetic field of the rotating, propagating ion beam to prevent the beam from expanding radially upon extraction

Beamline for low-energy transport of highly charged ions at HITRAP

International Nuclear Information System (INIS)

Andelkovic, Z.; Herfurth, F.; Kotovskiy, N.; König, K.; Maaß, B.; Murböck, T.; Neidherr, D.; Schmidt, S.; Steinmann, J.; Vogel, M.; Vorobjev, G.

2015-01-01

A beamline for transport of highly charged ions with energies as low as a few keV/charge has been constructed and commissioned at GSI. Complementary to the existing infrastructure of the HITRAP facility for deceleration of highly charged ions from the GSI accelerator, the new beamline connects the HITRAP ion decelerator and an EBIT with the associated experimental setups. Therefore, the facility can now transport the decelerated heavy highly charged ions to the experiments or supply them offline with medium-heavy highly charged ions from the EBIT, both at energies as low as a few keV/charge. Here we present the design of the 20 m long beamline with the corresponding beam instrumentation, as well as its performance in terms of energy and transport efficiency

High energy heavy ion beam lithography in silicon

International Nuclear Information System (INIS)

Rout, Bibhudutta; Dymnikov, Alexander D.; Zachry, Daniel P.; Eschenazi, Elia V.; Wang, Yongqiang Q.; Greco, Richard R.; Glass, Gary A.

2007-01-01

As high energy ions travel through a crystalline semiconductor materials they produce damage along the path which results in resistance to some of the wet chemical etching. A series of preliminary experiments have been performed at the Louisiana Accelerator Center (LAC) to examine the feasibility of irradiating high energy (keV-MeV) ions such as protons, xenon and gold through microscale masked structures on crystalline (n-type) Si substrates followed by wet chemical etch with KOH for attaining deep micromachining in Si. The results of these experiments are reported

Modified Thomson spectrometer design for high energy, multi-species ion sources

International Nuclear Information System (INIS)

Gwynne, D.; Kar, S.; Doria, D.; Ahmed, H.; Hanton, F.; Cerchez, M.; Swantusch, M.; Willi, O.; Fernandez, J.; Gray, R. J.; MacLellan, D. A.; McKenna, P.; Green, J. S.; Neely, D.; Najmudin, Z.; Streeter, M.; Ruiz, J. A.; Schiavi, A.; Zepf, M.; Borghesi, M.

2014-01-01

A modification to the standard Thomson parabola spectrometer is discussed, which is designed to measure high energy (tens of MeV/nucleon), broad bandwidth spectra of multi-species ions accelerated by intense laser plasma interactions. It is proposed to implement a pair of extended, trapezoidal shaped electric plates, which will not only resolve ion traces at high energies, but will also retain the lower energy part of the spectrum. While a longer (along the axis of the undeflected ion beam direction) electric plate design provides effective charge state separation at the high energy end of the spectrum, the proposed new trapezoidal shape will enable the low energy ions to reach the detector, which would have been clipped or blocked by simply extending the rectangular plates to enhance the electrostatic deflection

Heavy ion fragmentation in high energy

International Nuclear Information System (INIS)

Nemes, M.C.

1985-01-01

A review is made on the theoretical aspects of heavy ion collisions at high energies. A comparison with several experimental data obtained in a large variety of experiments is present. An emphasis is given on the basis of Glauber's theory of scattering. (L.C.) [pt

Mixing of phosphorus and antimony ions in silicon by recoil implantation

International Nuclear Information System (INIS)

Kwok, H.L.; Lam, Y.W.; Wong, S.P.; Poon, M.C.

1986-01-01

The effects of mixing phosphorus and antimony ions in silicon by recoil implantation were examined. The electrical properties after ion mixing were investigated, and the results were compared with those obtained using other techniques. Different degrees of activation were also studied, by investigating the annealing behaviour. (U.K.)

High energy ion implantation

International Nuclear Information System (INIS)

Ziegler, J.F.

1985-01-01

High energy ion implantation offers the oppertunity for unique structures in semiconductor processing. The unusual physical properties of such implantations are discussed as well as the special problems in masking and damage annealing. A review is made of proposed circuit structures which involve deep implantation. Examples are: deep buried bipolar collectors fabricated without epitaxy, barrier layers to reduce FET memory sensitivity to soft-fails, CMOS isolation well structures, MeV implantation for customization and correction of completed circuits, and graded reach-throughs to deep active device components. (orig.)

Fabricating high-energy quantum dots in ultra-thin LiFePO4 nanosheets using a multifunctional high-energy biomolecule-ATP

DEFF Research Database (Denmark)

Zhang, X.D.; Bi, Z.Y.; He, W.

2014-01-01

By using a multifunctional high-energy biomolecule—adenosine triphosphate (ATP)—we fabricated highenergy quantum dots (HEQDs) with a feature size of less than 10 nm and used them in high-power lithium-ion batteries. We introduced high-energy phosphate bonds into the crystal structure of LiFePO4...... nanoparticles and synthesized the mesoporous biocarbon nanowire coated LiFePO4 with HEQDs (MBCNW-LFP-HEQDs) by using ATP as a phosphorus source, a nucleating agent, a structural template and a biocarbon source. HEGDs were homogeneously formed inside the ultra-thin LiFePO4 nanosheet and the mesoporous biocarbon...... nanowire network structure was coated on the surface of the nanosheet. In LiFePO4 nanoparticles, HEQDs result in more storage sites of Li+ ions and easier transfer kinetics of electrons and lithium ions, where the kinetic transformation path between LiFePO4 and FePO4 is rather different from the path...

Numerical analysis of energy density and particle density in high energy heavy-ion collisions

International Nuclear Information System (INIS)

Fu Yuanyong; Lu Zhongdao

2004-01-01

Energy density and particle density in high energy heavy-ion collisions are calculated with infinite series expansion method and Gauss-Laguerre formulas in numerical integration separately, and the results of these two methods are compared, the higher terms and linear terms in series expansion are also compared. The results show that Gauss-Laguerre formulas is a good method in calculations of high energy heavy-ion collisions. (author)

Reaction mechanism in high energy heavy-ion collisions

International Nuclear Information System (INIS)

Tanihata, Isao.

1982-04-01

The reaction mechanism in high energy heavy-ion collision is discussed. The discussion is mainly based on the experimental data. Empirical equations have been given for the total cross-sections of nucleus-nucleus reactions and the reaction cross-sections. These cross-sections are well described by the geometrical size of the colliding nuclei. The cross-sections are also understood by microscopic calculation. The charged particle multiplicity gives additional information about the geometrical aspect of heavy ion collision. The data suggested that the total energy, independent of projectile size, is most important for determining the multiplicity. The inclusive proton spectrum in a heavy ion collision showed two distinct regions. The one is the fragment region, and the other the participant region. The spectral shapes of inclusive pion spectra are reasonably well explained by the Coulomb interaction of pions with nuclear fragments. The high energy heavy ion reaction occurs in the overlap region of the projectile and target. This has been tested by measuring the number of participants for various reactions. The space and the time structure of the collision are also discussed in this paper as well as the dynamical aspects of the collision. (Kato, T.)

High Energy Ion Bombardment Simulation Facility at the University of Pittsburgh

International Nuclear Information System (INIS)

McGruer, J.N.; Choyke, W.J.; Doyle, N.J.; Spitznagel, J.A.

1975-01-01

The High Energy Ion Bombardment Simulation (HEIBS) Facility located at the University of Pittsburgh is now operational. The E-22 tandem accelerator of the Nuclear Physics Laboratory, fitted with a UNIS source, provides the heavy high energy ions. An auxiliary Van de Graaff accelerator is used for the simultaneous production of He ions. Special features of the simulation laboratory are reported

Geometric and electronic structures of molecular ions from high energy collisions

International Nuclear Information System (INIS)

Groeneveld, K.O.

1983-01-01

This chapter examines the characteristics of heavy ion collision and of beam foil spectroscopy. It discusses the kinematic consequences of the high energies and presents results from ''Coulomb explosion'' and structure determination of molecular ions. It demonstrates that studies of molecular ions with accelerators can provide electronic and geometric structure information of molecules or molecular ions and points out that the understanding of the microscopic processes at such high energies is incomplete and needs further experimental and theoretical efforts

New aspects of high energy heavy-ion transfer reactions

International Nuclear Information System (INIS)

Scott, D.K.

1975-03-01

New aspects of heavy ion reactions at incident energies in the region of 10 MeV/nucleon are discussed with an emphasis on the peripheral nature of the collisions, which leads to simplicities in the differential cross sections. The distortion of the peripheral distribution through the interference of direct and multistep processes is used to illustrate aspects of high energy reactions unique to heavy ions. The simplicities of the distributions for reactions on lighter nuclei are exploited to give new information about nuclear structure from direct and compound reactions at high energy. (16 figures, 32 references) (U.S.)

Experiments on very high energy heavy ions

International Nuclear Information System (INIS)

Willis, W.J.

1981-01-01

In this paper I describe experimental techniques which could be used to investigate central collision of very high energy heavy ions. For my purposes, the energy range is defined by the number of pions produced, Nsub(π) >> 100, and consequently Nsub(π) >> Nsub(nucleon). In this regime we may expect that new phenomena will appear. (orig.)

Nonlinear energy loss of highly charged heavy ions

International Nuclear Information System (INIS)

Zwicknagel, G.Guenter.

2000-01-01

For slow, highly charged heavy ions strong coupling effects in the energy transfer from the projectile-ion to an electron target plasma become important. A theoretical description of this nonlinear ion stopping has to go beyond the standard approaches like the dielectric linear response or the binary collision model which are strictly valid only at weak ion-target coupling. Here we outline an improved treatment which is based on a suitable combination of binary collision and linear response contributions. As has been verified for isotropic, nonmagnetized electron plasmas by comparison with simulations, this approach well reproduces the essential features of nonlinear stopping up to moderate coupling strength. Its extension to anisotropic, magnetized electron plasmas basically involves the fully numerical determination of the momentum and energy transfer in binary ion-electron collisions in the presence of a magnetic field. First results of such calculations are presented and discussed

Ion induced high energy electron emission from copper

International Nuclear Information System (INIS)

Ruano, G.; Ferron, J.

2008-01-01

We present measurements of secondary electron emission from Cu induced by low energy bombardment (1-5 keV) of noble gas (He + , Ne + and Ar + ) and Li + ions. We identify different potential and kinetic mechanisms and find the presence of high energetic secondary electrons for a couple of ion-target combinations. In order to understand the presence of these fast electrons we need to consider the Fermi shuttle mechanism and the different ion neutralization efficiencies.

Ion induced high energy electron emission from copper

Energy Technology Data Exchange (ETDEWEB)

Ruano, G. [Instituto de Desarrollo Tecnologico para la Industria Quimica, Consejo Nacional de Investigaciones Cientificas y Tecnicas and Universidad Nacional del Litoral Gueemes 3450 CC 91, 3000 Santa Fe (Argentina)], E-mail: gdruano@ceride.gov.ar; Ferron, J. [Instituto de Desarrollo Tecnologico para la Industria Quimica, Consejo Nacional de Investigaciones Cientificas y Tecnicas and Universidad Nacional del Litoral Gueemes 3450 CC 91, 3000 Santa Fe (Argentina); Departamento de Ingenieria de Materiales, Facultad de Ingenieria Quimica, Consejo Nacional de Investigaciones Cientificas y Tecnicas and Universidad Nacional del Litoral Gueemes 3450 CC 91, 3000 Santa Fe (Argentina)

2008-11-15

We present measurements of secondary electron emission from Cu induced by low energy bombardment (1-5 keV) of noble gas (He{sup +}, Ne{sup +} and Ar{sup +}) and Li{sup +} ions. We identify different potential and kinetic mechanisms and find the presence of high energetic secondary electrons for a couple of ion-target combinations. In order to understand the presence of these fast electrons we need to consider the Fermi shuttle mechanism and the different ion neutralization efficiencies.

[Effects of phosphorus sources on phosphorus fractions in rhizosphere soil of wild barley genotypes with high phosphorus utilization efficiency].

Science.gov (United States)

Cai, Qiu-Yan; Zhang, Xi-Zhou; Li, Ting-Xuan; Chen, Guang-Deng

2014-11-01

High P-efficiency (IS-22-30, IS-22-25) and low P-efficiency (IS-07-07) wild barley cultivars were chosen to evaluate characteristics of phosphorus uptake and utilization, and properties of phosphorus fractions in rhizosphere and non-rhizosphere in a pot experiment with 0 (CK) and 30 mg P · kg(-1) supplied as only Pi (KH2PO4), only Po (phytate) or Pi + Po (KH2PO4+ phytate). The results showed that dry matter and phosphorus accumulation of wild barley in the different treatments was ranked as Pi > Pi + Po > Po > CK. In addition, dry matter yield and phosphorus uptake of wild barley with high P-efficiency exhibited significantly greater than that with low P-efficiency. The concentration of soil available phosphorus was significantly different after application of different phosphorus sources, which was presented as Pi > Pi + Po > Po. The concentration of soil available phosphorus in high P-efficiency wild barley was significantly higher than that of low P-efficiency in the rhizosphere soil. There was a deficit in rhizosphere available phosphorus of high P-efficiency wild barley, especially in Pi and Pi+Po treatments. The inorganic phosphorus fractions increased with the increasing Pi treatment, and the concentrations of inorganic phosphorus fractions in soil were sorted as follows: Ca10-P > O-P > Fe-P > Al-P > Ca2-P > Ca8-P. The contents of Ca2-P and Ca8-P for high P-efficiency wild barley showed deficits in rhizosphere soil under each phosphorus source treatment. In addition, enrichment of Al-P and Fe-P was observed in Pi treatment in rhizosphere soil. The concentrations of organic phosphorus fractions in soil were sorted as follows: moderate labile organic phosphorus > moderate resistant, resistant organic phosphorus > labile organic phosphorus. The labile and moderate labile organic phosphorus enriched in rhizosphere soil and the greatest enrichment appeared in Pi treatment. Furthermore, the concentrations of moderate resistant organic phosphorus and resistant

High energy metal ion implantation using 'Magis', a novel, broad-beam, Marx-generator-based ion source

International Nuclear Information System (INIS)

Anders, A.; Brown, I.G.; Dickinson, M.R.; MacGill, R.A.

1996-08-01

Ion energy of the beam formed by an ion source is proportional to extractor voltage and ion charge state. Increasing the voltage is difficult and costly for extraction voltage over 100 kV. Here we explore the possibility of increasing the charge states of metal ions to facilitate high-energy, broad beam ion implantation at a moderate voltage level. Strategies to enhance the ion charge state include operating in the regimes of high-current vacuum sparks and short pulses. Using a time-of-flight technique we have measured charge states as high as 7+ (73 kA vacuum spark discharge) and 4+ (14 kA short pulse arc discharge), both for copper, with the mean ion charge states about 6.0 and 2.5, respectively. Pulsed discharges can conveniently be driven by a modified Marx generator, allowing operation of ''Magis'' with a single power supply (at ground potential) for both plasma production and ion extraction

Energy and Pitch Distribution of Spontaneously-generated High-energy Bulk Ions in the RFP

Science.gov (United States)

Kim, Jungha; Anderson, Jay; Reusch, Joshua; Eilerman, Scott; Capecchi, William

2014-10-01

Magnetic reconnection events in the reversed field pinch (RFP) are known to heat bulk and impurity ions. Runaway due to a parallel electric field has recently been confirmed as an important acceleration mechanism for high energy test ions supplied by a neutral beam. This effect does not, however, explain the change in distribution of nearly Maxwellian bulk ions at a reconnection event. By operating MST near maximum current and low electron density, significant fusion neutron flux can be generated without neutral beam injection. The bulk ion distribution created in these plasmas is well-confined, non-Maxwellian, and can be measured by the Advanced Neutral Particle Analyzer (ANPA) placed at a radial or tangential porthole. Data show a high energy tail up to 25 keV with a relatively higher signal in the low energy channels (8-15 keV) at the radial port following a reconnection event. Analysis of the energy dependence of trapped orbits sampled by the ANPA at the radial view implies an abundance of lower energy particles in regions of higher neutral density. This mandates a careful deconvolution of the measured ANPA signal to compute the fast ion distribution. This work is supported by the US DOE and NSF.

Emission of high-energy, light particles from intermediate-energy heavy-ion reactions

International Nuclear Information System (INIS)

Ball, J.B.; Auble, R.L.

1982-01-01

One of the early surprises in examining reaction products from heavy ion reactions at 10 MeV/nucleon and above was the large yield of light particles emitted and the high energies to which the spectra of these particles extended. The interpretation of the origin of the high energy light ions has evolved from a picture of projectile excitation and subsequent evaporation to one of pre-equilibrium (or nonequilibrium) emission. The time scale for particle emission has thus moved from one that occurs following the initial collision to one that occurs at the very early stages of the collision. Research at ORNL on this phenomenon is reviewed

High energy ion implantation for IC processing

International Nuclear Information System (INIS)

Oosterhoff, S.

1986-01-01

In this thesis the results of fundamental research on high energy ion implantation in silicon are presented and discussed. The implantations have been carried out with the 500 kV HVEE ion implantation machine, that was acquired in 1981 by the IC technology and Electronics group at Twente University of Technology. The damage and anneal behaviour of 1 MeV boron implantations to a dose of 10 13 /cm 2 have been investigated as a function of anneal temperature by sheet resistance, Hall and noise measurements. (Auth.)

Development of a CMOS process using high energy ion implantation

International Nuclear Information System (INIS)

Stolmeijer, A.

1986-01-01

The main interest of this thesis is the use of complementary metal oxide semiconductors (CMOS) in electronic technology. Problems in developing a CMOS process are mostly related to the isolation well of p-n junctions. It is shown that by using high energy ion implantation, it is possible to reduce lateral dimensions to obtain a rather high packing density. High energy ion implantation is also presented as a means of simplifying CMOS processing, since extended processing steps at elevated temperatures are superfluous. Process development is also simplified. (Auth.)

Interaction of low-energy highly charged ions with matter

International Nuclear Information System (INIS)

Ginzel, Rainer

2010-01-01

The thesis presented herein deals with experimental studies of the interaction between highly charged ions and neutral matter at low collision energies. The energy range investigated is of great interest for the understanding of both charge exchange reactions between ions comprising the solar wind and various astrophysical gases, as well as the creation of near-surface nanostructures. Over the course of this thesis an experimental setup was constructed, capable of reducing the kinetic energy of incoming ions by two orders of magnitude and finally focussing the decelerated ion beam onto a solid or gaseous target. A coincidence method was employed for the simultaneous detection of photons emitted during the charge exchange process together with the corresponding projectile ions. In this manner, it was possible to separate reaction channels, whose superposition presumably propagated large uncertainties and systematic errors in previous measurements. This work has unveiled unexpectedly strong contributions of slow radiative decay channels and clear evidence of previously only postulated decay processes in charge exchange-induced X-ray spectra. (orig.)

Inverted end-Hall-type low-energy high-current gaseous ion source

International Nuclear Information System (INIS)

Oks, E. M.; Vizir, A. V.; Shandrikov, M. V.; Yushkov, G. Yu.; Grishin, D. M.; Anders, A.; Baldwin, D. A.

2008-01-01

A novel approach to low-energy, high-current, gaseous ion beam generation was explored and an ion source based on this technique has been developed. The source utilizes a dc high-current (up to 20 A) gaseous discharge with electron injection into the region of ion generation. Compared to the conventional end-Hall ion source, the locations of the discharge anode and cathode are inverted: the cathode is placed inside the source and the anode outside, and correspondingly, the discharge current is in the opposite direction. The discharge operates in a diverging axial magnetic field, similar to the end-Hall source. Electron generation and injection is accomplished by using an additional arc discharge with a ''cold'' (filamentless) hollow cathode. Low plasma contamination is achieved by using a low discharge voltage (avoidance of sputtering), as well as by a special geometric configuration of the emitter discharge electrodes, thereby filtering (removing) the erosion products stemming from the emitter cathode. The device produces a dc ion flow with energy below 20 eV and current up to 2.5 A onto a collector of 500 cm 2 at 25 cm from the source edge, at a pressure ≥0.02 Pa and gas flow rate ≥14 SCCM. The ion energy spread is 2 to 3 eV (rms). The source is characterized by high reliability, low maintenance, and long lifetime. The beam contains less than 0.1% of metallic ions. The specific electric energy consumption is 400 eV per ion registered at the collector. The source operates with noble gases, nitrogen, oxygen, and hydrocarbons. Utilizing biasing, it can be used for plasma sputtering, etching, and other ion technologies

Transverse microanalysis of high energy Ion implants

Energy Technology Data Exchange (ETDEWEB)

Dooley, S.P.; Jamieson, D.N.; Nugent, K.W.; Prawer, S. [Melbourne Univ., Parkville, VIC (Australia). School of Physics

1996-12-31

High energy ion implants in semiconductor materials have been analyzed by Channeling Contrast Microscopy (CCM) perpendicular to the implant direction, allowing imaging of the entire ion track. The damage produced by Channeled and Random 1.4 MeV H{sup +} implants into the edge of a <100> type IIa diamond wafer were analyzed by channeling into the face of the crystal. The results showed negligible damage in the surface region of the implants, and swelling induced misalignment at the end of range of the implants. Channeled 1.4 MeV H{sup +} implants in diamond had a range only 9% deeper than Random implants, which could be accounted for by dechanneling of the beam. The channeling of H{sup +}{sub 2} ions has been previously found to be identical to that of protons of half energy, however the current experiment has shown a 1% increase in {chi}{sub min} for H{sup +}{sub 2} in diamond compared to H{sup +} at 1,2 MeV per proton. This is due to repulsion between protons within the same channel. 5 refs., 2 figs.

Transverse microanalysis of high energy Ion implants

Energy Technology Data Exchange (ETDEWEB)

Dooley, S P; Jamieson, D N; Nugent, K W; Prawer, S [Melbourne Univ., Parkville, VIC (Australia). School of Physics

1997-12-31

High energy ion implants in semiconductor materials have been analyzed by Channeling Contrast Microscopy (CCM) perpendicular to the implant direction, allowing imaging of the entire ion track. The damage produced by Channeled and Random 1.4 MeV H{sup +} implants into the edge of a <100> type IIa diamond wafer were analyzed by channeling into the face of the crystal. The results showed negligible damage in the surface region of the implants, and swelling induced misalignment at the end of range of the implants. Channeled 1.4 MeV H{sup +} implants in diamond had a range only 9% deeper than Random implants, which could be accounted for by dechanneling of the beam. The channeling of H{sup +}{sub 2} ions has been previously found to be identical to that of protons of half energy, however the current experiment has shown a 1% increase in {chi}{sub min} for H{sup +}{sub 2} in diamond compared to H{sup +} at 1,2 MeV per proton. This is due to repulsion between protons within the same channel. 5 refs., 2 figs.

Investigation of structural materials of reactors using high-energy heavy-ion irradiations

International Nuclear Information System (INIS)

Wang Zhiguang

2007-01-01

Radiation damage in structural materials of fission/fusion reactors is mainly attributed to the evolution of intensive atom displacement damage induced by energetic particles (n, α and/or fission fragments) and high-rate helium doping by direct α particle bombardments and/or (n, α) reactions. It can cause severe degradation of reactor structural materials such as surface blistering, bulk void swelling, deformation, fatigue, embrittlement, stress erosion corrosion and so on that will significantly affect the operation safety of reactors. However, up to now, behavior of structural materials at the end of their service can hardly be fully tested in a real reactor. In the present work, damage process in reactor structural materials is briefly introduced, then the advantages of energetic ion implantation/irradiation especially high-energy heavy ion irradiation are discussed, and several typical examples on simulation of radiation effects in reactor candidate structural materials using high-energy heavy ion irradiations are pronounced. Experimental results and theoretical analysis suggested that irradiation with energetic particles especially high-energy heavy ions is very useful technique for simulating the evolution of microstructures and macro-properties of reactor structural materials. Furthermore, an on-going plan of material irradiation experiments using high energy H- and He-ions based on the Heavy Ion Research Facilities in Lanzhou (HIRFL) is also briefly interpreted. (authors)

An intranuclear cascade calculation of high-energy heavy-ion interactions

International Nuclear Information System (INIS)

Yariv, Y.; Fraenkel, Z.

1979-01-01

The intranuclear cascade model of Chen is extended to high-energy reactions between two heavy ions. The results of the calculations are compared with experimental results for the inclusive proton and pion cross sections, two-particle correlations, particle multiplicity distributions and spallation cross section distributions from light ( 12 C+ 12 C) to heavy( 40 Ar + 238 U) projectile-target systems in the laboratory bombarding energy range E/A=250-1000 MeV. The comparison shows that the model is fairly successful in reproducing the various aspects of high-energy reactions between heavy ions. It is also shown that the assumption that high particle multiplicities are indicative of ''central'' (small impact parameter) collisions are well founded for heavy projectile-target systems. (B.G.)

Toward Low-Cost, High-Energy Density, and High-Power Density Lithium-Ion Batteries

Science.gov (United States)

Li, Jianlin; Du, Zhijia; Ruther, Rose E.; AN, Seong Jin; David, Lamuel Abraham; Hays, Kevin; Wood, Marissa; Phillip, Nathan D.; Sheng, Yangping; Mao, Chengyu; Kalnaus, Sergiy; Daniel, Claus; Wood, David L.

2017-09-01

Reducing cost and increasing energy density are two barriers for widespread application of lithium-ion batteries in electric vehicles. Although the cost of electric vehicle batteries has been reduced by 70% from 2008 to 2015, the current battery pack cost (268/kWh in 2015) is still >2 times what the USABC targets (125/kWh). Even though many advancements in cell chemistry have been realized since the lithium-ion battery was first commercialized in 1991, few major breakthroughs have occurred in the past decade. Therefore, future cost reduction will rely on cell manufacturing and broader market acceptance. This article discusses three major aspects for cost reduction: (1) quality control to minimize scrap rate in cell manufacturing; (2) novel electrode processing and engineering to reduce processing cost and increase energy density and throughputs; and (3) material development and optimization for lithium-ion batteries with high-energy density. Insights on increasing energy and power densities of lithium-ion batteries are also addressed.

Shielding experiments with high-energy heavy ions for spaceflight applications

International Nuclear Information System (INIS)

Zeitlin, C; Guetersloh, S; Heilbronn, L; Miller, J; Elkhayari, N; Empl, A; LeBourgeois, M; Mayes, B W; Pinsky, L; Christl, M; Kuznetsov, E

2008-01-01

Mitigation of radiation exposures received by astronauts on deep-space missions must be considered in the design of future spacecraft. The galactic cosmic rays (GCR) include high-energy heavy ions, many of which have ranges that exceed the depth of shielding that can be launched in realistic scenarios. Some of these ions are highly ionizing (producing a high dose per particle) and for some biological endpoints are more damaging per unit dose than sparsely ionizing radiation. The principal physical mechanism by which the dose and dose equivalent delivered by these particles can be reduced is nuclear fragmentation, the result of inelastic collisions between nuclei in the hull of the spacecraft and/or other materials. These interactions break the incident ions into lighter, less ionizing and less biologically effective particles. We have previously reported the tests of shielding effectiveness using many materials in a 1 GeV nucleon -1 56 Fe beam, and also reported results using a single polyethylene (CH 2 ) target in a variety of beam ions and energies up to 1 GeV nucleon -1 . An important, but tentative, conclusion of those studies was that the average behavior of heavy ions in the GCR would be better simulated by heavy beams at energies above 1 GeV nucleon -1 . Following up on that work, we report new results using beams of 12 C, 28 Si and 56 Fe, each at three energies, 3, 5 and 10 GeV nucleon -1 , on carbon, polyethylene, aluminium and iron targets

Shielding experiments with high-energy heavy ions for spaceflight applications

Energy Technology Data Exchange (ETDEWEB)

Zeitlin, C; Guetersloh, S; Heilbronn, L; Miller, J [Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Elkhayari, N; Empl, A; LeBourgeois, M; Mayes, B W; Pinsky, L [Physics Department, University of Houston, Houston, TX (United States); Christl, M [NASA Marshall Spaceflight Center, Huntsville, AL (United States); Kuznetsov, E [Physics Department, University of Alabama, Huntsville, AL (United States)], E-mail: cjzeitlin@lbl.gov

2008-07-15

Mitigation of radiation exposures received by astronauts on deep-space missions must be considered in the design of future spacecraft. The galactic cosmic rays (GCR) include high-energy heavy ions, many of which have ranges that exceed the depth of shielding that can be launched in realistic scenarios. Some of these ions are highly ionizing (producing a high dose per particle) and for some biological endpoints are more damaging per unit dose than sparsely ionizing radiation. The principal physical mechanism by which the dose and dose equivalent delivered by these particles can be reduced is nuclear fragmentation, the result of inelastic collisions between nuclei in the hull of the spacecraft and/or other materials. These interactions break the incident ions into lighter, less ionizing and less biologically effective particles. We have previously reported the tests of shielding effectiveness using many materials in a 1 GeV nucleon{sup -1} {sup 56}Fe beam, and also reported results using a single polyethylene (CH{sub 2}) target in a variety of beam ions and energies up to 1 GeV nucleon{sup -1}. An important, but tentative, conclusion of those studies was that the average behavior of heavy ions in the GCR would be better simulated by heavy beams at energies above 1 GeV nucleon{sup -1}. Following up on that work, we report new results using beams of {sup 12}C, {sup 28}Si and {sup 56}Fe, each at three energies, 3, 5 and 10 GeV nucleon{sup -1}, on carbon, polyethylene, aluminium and iron targets.

Nanometer-size surface modification produced by single, low energy, highly charged ions

International Nuclear Information System (INIS)

Stockli, M.P.

1994-01-01

Atomically flat surfaces of insulators have been bombarded with low energy, highly charged ions to search for nanometer-size surface modifications. It is expected that the high electron deficiency of highly charged ions will capture and/or remove many of the insulator's localized electrons when impacting on an insulating surface. The resulting local electron deficiency is expected to locally disintegrate the insulator through a open-quotes Coulomb explosionclose quotes forming nanometer-size craters. Xe ions with charge states between 10+ and 45+ and kinetic energies between 0 and 10 keV/q were obtained from the KSU-CRYEBIS, a CRYogenic Electron Beam Ion Source and directed onto various insulating materials. Mica was favored as target material as atomically flat surfaces can be obtained reliably through cleaving. However, the authors observations with an atomic force microscope have shown that mica tends to defoliate locally rather than disintegrate, most likely due to the small binding forces between adjacent layers. So far the authors measurements indicate that each ion produces one blister if the charge state is sufficiently high. The blistering does not seem to depend very much on the kinetic energy of the ions

The interactions of high-energy, highly-charged ions with fullerenes

International Nuclear Information System (INIS)

Ali, R.; Berry, H.G.; Cheng, S.

1996-01-01

In 1985, Robert Curl and Richard Smalley discovered a new form of carbon, the fullerene, C 60 , which consists of 60 carbon atoms in a closed cage resembling a soccer ball. In 1990, Kritschmer et al. were able to make macroscopic quantities of fullerenes. This has generated intense activity to study the properties of fullerenes. One area of research involves collisions between fullerenes and atoms, ions or electrons. In this paper we describe experiments involving interactions between fullerenes and highly charged ions in which the center-of-mass energies exceed those used in other work by several orders of magnitude. The high values of projectile velocity and charge state result in excitation and decay processes differing significantly from those seen in studies 3 at lower energies. Our results are discussed in terms of theoretical models analogous to those used in nuclear physics and this provides an interesting demonstration of the unity of physics

Development of high current low energy H+ ion source

International Nuclear Information System (INIS)

Forrester, A.T.; Crow, J.T.; Goebel, D.M.

1978-01-01

The ultimate goal of this work is the development of an ion source suitable for double charge exchange of D + ions to D - ions in cesium or other vapor. Since the fraction of the D + which changes to D - may be as high as 0.35 in the energy below one keV, the process appears very favorable. What is desired is a source of several hundred cm 2 area, with a D + current density greater than, say 0.2A/cm 2 . Small angular spread is essential with up to about 0.1 radian being acceptable. A simple approach to this problem appears to be through fine mesh extraction electrodes. In this system a single grid facing the ion source plasma constitutes the entire extraction electrode system. If the potential difference between the grid and the source plasma is large compared to the ion energy at the plasma boundary, then the distance s 0 is just the Child-Langmuir distance corresponding to the ion current density J and the potential difference V 0 between the plasma and the grid

Electrical properties of InP:Fe single crystals implanted by phosphorus ions

International Nuclear Information System (INIS)

Radautsan, S.I.; Tiginyanu, I.M.; Pyshnaya, N.B.

1988-01-01

Investigations of phosphorus ion implantation in InP:Fe monocrystals and of the post-implantation annealing process upon the electrical properties of InP:Fe were carried out. The electrical parameters of the samples have been determined by Hall effect measurements. The curves of electron surface concentration n s and mobility μ s as functions of annealing temperature in the range of 200 to 600 0 C are shown and discussed. In order to estimate the depth of donor levels in annealed samples the temperature dependence of the surface Hall coefficient has been studied in the range 100 to 400 K. The thermal electron activation energy has been determined to be 0.09 eV

Live cell imaging combined with high-energy single-ion microbeam

Science.gov (United States)

Guo, Na; Du, Guanghua; Liu, Wenjing; Guo, Jinlong; Wu, Ruqun; Chen, Hao; Wei, Junzhe

2016-03-01

DNA strand breaks can lead to cell carcinogenesis or cell death if not repaired rapidly and efficiently. An online live cell imaging system was established at the high energy microbeam facility at the Institute of Modern Physics to study early and fast cellular response to DNA damage after high linear energy transfer ion radiation. The HT1080 cells expressing XRCC1-RFP were irradiated with single high energy nickel ions, and time-lapse images of the irradiated cells were obtained online. The live cell imaging analysis shows that strand-break repair protein XRCC1 was recruited to the ion hit position within 20 s in the cells and formed bright foci in the cell nucleus. The fast recruitment of XRCC1 at the ion hits reached a maximum at about 200 s post-irradiation and then was followed by a slower release into the nucleoplasm. The measured dual-exponential kinetics of XRCC1 protein are consistent with the proposed consecutive reaction model, and the measurements obtained that the reaction rate constant of the XRCC1 recruitment to DNA strand break is 1.2 × 10-3 s-1 and the reaction rate constant of the XRCC1 release from the break-XRCC1 complex is 1.2 × 10-2 s-1.

Energy loss and charge exchange processes of high energy heavy ions channeled in crystals

International Nuclear Information System (INIS)

Poizat, J.C.; Andriamonje, S.; Anne, R.; Faria, N.V.d.C.; Chevallier, M.; Cohen, C.; Dural, J.; Farizon-Mazuy, B.; Gaillard, M.J.; Genre, R.; Hage-Ali, M.; Kirsch, R.; L'hoir, A.; Mory, J.; Moulin, J.; Quere, Y.; Remillieux, J.; Schmaus, D.; Toulemonde, M.

1990-01-01

The interaction of moving ions with single crystals is very sensitive to the orientation of the incident beam with respect to the crystalline directions of the target. Our experiments show that high energy heavy ion channeling deeply modifies their slowing down and charge exchange processes. This is due to the fact that channeled ions interact only with outershell target electrons, which means that the electron density they experience is very low and that the binding energy, and then the momentum distribution of these electrons, are quite different from the corresponding average values associated to random incidence. The two experimental studies presented here show the reduction of the energy loss rate for fast channeled heavy ions and illustrate the two aspects of channeling effects on charge exchange, the reduction of electron loss on one hand, and of electron capture on the other hand

Ultrathin and Ion-Selective Janus Membranes for High-Performance Osmotic Energy Conversion.

Science.gov (United States)

Zhang, Zhen; Sui, Xin; Li, Pei; Xie, Ganhua; Kong, Xiang-Yu; Xiao, Kai; Gao, Longcheng; Wen, Liping; Jiang, Lei

2017-07-05

The osmotic energy existing in fluids is recognized as a promising "blue" energy source that can help solve the global issues of energy shortage and environmental pollution. Recently, nanofluidic channels have shown great potential for capturing this worldwide energy because of their novel transport properties contributed by nanoconfinement. However, with respect to membrane-scale porous systems, high resistance and undesirable ion selectivity remain bottlenecks, impeding their applications. The development of thinner, low-resistance membranes, meanwhile promoting their ion selectivity, is a necessity. Here, we engineered ultrathin and ion-selective Janus membranes prepared via the phase separation of two block copolymers, which enable osmotic energy conversion with power densities of approximately 2.04 W/m 2 by mixing natural seawater and river water. Both experiments and continuum simulation help us to understand the mechanism for how membrane thickness and channel structure dominate the ion transport process and overall device performance, which can serve as a general guiding principle for the future design of nanochannel membranes for high-energy concentration cells.

Modification of high density polyethylene by gold implantation using different ion energies

Energy Technology Data Exchange (ETDEWEB)

Nenadović, M.; Potočnik, J. [INS Vinca, Laboratory of Atomic Physics, University of Belgrade, Mike Alasa 12–14, 11001 Belgrade (Serbia); Mitrić, M. [INS Vinca, Condensed Matter Physics Laboratory, University of Belgrade, Mike Alasa 12–14, 11001 Belgrade (Serbia); Štrbac, S. [ICTM Institute of Electrochemistry, University of Belgrade, Njegoseva 12, 11001 Belgrade (Serbia); Rakočević, Z., E-mail: zlatkora@vinca.rs [INS Vinca, Laboratory of Atomic Physics, University of Belgrade, Mike Alasa 12–14, 11001 Belgrade (Serbia)

2013-11-01

High density polyethylene (HDPE) samples were modified by Au{sup +} ion implantation at a dose of 5 × 10{sup 15} ions cm{sup −2}, using energies of 50, 100, 150 and 200 keV. The existence of implanted gold in the near-surface region of HDPE samples was confirmed by X-ray diffraction analysis. Surface roughness and Power Spectral Density analyses based on Atomic Force Microscopy (AFM) images of the surface topography revealed that the mechanism of HDPE modification during gold ion implantation depended on the energy of gold ions. Histograms obtained from phase AFM images indicated a qualitative change in the chemical composition of the surface during implantation with gold ions with different energies. Depth profiles obtained experimentally from cross-sectional Force Modulation Microscopy images and ones obtained from a theoretical simulation are in agreement for gold ions energies lower than 100 keV. The deviation that was observed for higher energies of the gold ions is explained by carbon precipitation in the near surface region of the HDPE, which prevented the penetration of gold ions further into the depth of the sample. - Highlights: • HDPE was implanted by Au{sup +} ions using energies of 50, 100, 150 and 200 keV. • Surface composition was analyzed from phase AFM images. • FMM depth profiles are in agreement with theoretical ones for energies up to 100 keV. • A deviation is observed for higher gold ion energies.

Modification of high density polyethylene by gold implantation using different ion energies

International Nuclear Information System (INIS)

Nenadović, M.; Potočnik, J.; Mitrić, M.; Štrbac, S.; Rakočević, Z.

2013-01-01

High density polyethylene (HDPE) samples were modified by Au + ion implantation at a dose of 5 × 10 15 ions cm −2 , using energies of 50, 100, 150 and 200 keV. The existence of implanted gold in the near-surface region of HDPE samples was confirmed by X-ray diffraction analysis. Surface roughness and Power Spectral Density analyses based on Atomic Force Microscopy (AFM) images of the surface topography revealed that the mechanism of HDPE modification during gold ion implantation depended on the energy of gold ions. Histograms obtained from phase AFM images indicated a qualitative change in the chemical composition of the surface during implantation with gold ions with different energies. Depth profiles obtained experimentally from cross-sectional Force Modulation Microscopy images and ones obtained from a theoretical simulation are in agreement for gold ions energies lower than 100 keV. The deviation that was observed for higher energies of the gold ions is explained by carbon precipitation in the near surface region of the HDPE, which prevented the penetration of gold ions further into the depth of the sample. - Highlights: • HDPE was implanted by Au + ions using energies of 50, 100, 150 and 200 keV. • Surface composition was analyzed from phase AFM images. • FMM depth profiles are in agreement with theoretical ones for energies up to 100 keV. • A deviation is observed for higher gold ion energies

High-intensity low energy titanium ion implantation into zirconium alloy

Science.gov (United States)

Ryabchikov, A. I.; Kashkarov, E. B.; Pushilina, N. S.; Syrtanov, M. S.; Shevelev, A. E.; Korneva, O. S.; Sutygina, A. N.; Lider, A. M.

2018-05-01

This research describes the possibility of ultra-high dose deep titanium ion implantation for surface modification of zirconium alloy Zr-1Nb. The developed method based on repetitively pulsed high intensity low energy titanium ion implantation was used to modify the surface layer. The DC vacuum arc source was used to produce metal plasma. Plasma immersion titanium ions extraction and their ballistic focusing in equipotential space of biased electrode were used to produce high intensity titanium ion beam with the amplitude of 0.5 A at the ion current density 120 and 170 mA/cm2. The solar eclipse effect was used to prevent vacuum arc titanium macroparticles from appearing in the implantation area of Zr sample. Titanium low energy (mean ion energy E = 3 keV) ions were implanted into zirconium alloy with the dose in the range of (5.4-9.56) × 1020 ion/cm2. The effect of ion current density, implantation dose on the phase composition, microstructure and distribution of elements was studied by X-ray diffraction, scanning electron microscopy and glow-discharge optical emission spectroscopy, respectively. The results show the appearance of Zr-Ti intermetallic phases of different stoichiometry after Ti implantation. The intermetallic phases are transformed from both Zr0.7Ti0.3 and Zr0.5Ti0.5 to single Zr0.6Ti0.4 phase with the increase in the implantation dose. The changes in phase composition are attributed to Ti dissolution in zirconium lattice accompanied by the lattice distortions and appearance of macrostrains in intermetallic phases. The depth of Ti penetration into the bulk of Zr increases from 6 to 13 μm with the implantation dose. The hardness and wear resistance of the Ti-implanted zirconium alloy were increased by 1.5 and 1.4 times, respectively. The higher current density (170 mA/cm2) leads to the increase in the grain size and surface roughness negatively affecting the tribological properties of the alloy.

A Hierarchy of Transport Approximations for High Energy Heavy (HZE) Ions

Science.gov (United States)

Wilson, John W.; Lamkin, Stanley L.; Hamidullah, Farhat; Ganapol, Barry D.; Townsend, Lawrence W.

1989-01-01

The transport of high energy heavy (HZE) ions through bulk materials is studied neglecting energy dependence of the nuclear cross sections. A three term perturbation expansion appears to be adequate for most practical applications for which penetration depths are less than 30 g per sq cm of material. The differential energy flux is found for monoenergetic beams and for realistic ion beam spectral distributions. An approximate formalism is given to estimate higher-order terms.

Ion trapping in the high-energy storage ring HESR

Energy Technology Data Exchange (ETDEWEB)

Hinterberger, Frank [Bonn Univ. (Germany). Helmholtz-Institut fuer Strahlen- und Kernphysik

2011-10-15

The problem of ion trapping in the high-energy storage ring HESR is studied in the present report. Positive ions are trapped in the negative potential well of the antiproton beam. The ions are produced by the interaction between the antiproton beam and the residual gas. The adverse effects of ion trapping like tune shifts, tune spreads and coherent instabilities are reviewed. The ion production rate by ionization of the residual gas molecules is estimated. The negative potential well and the corresponding electric fields of the antiproton beam are evaluated in order to study the transverse and longitudinal motion of the ions and the accumulation in trapping pockets. The removal of ions can be achieved using clearing electrodes and under certain conditions resonant transverse beam shaking. Diagnostic tools and measurements of trapped ion effects are sketched. (orig.)

Time of Flight based diagnostics for high energy laser driven ion beams

Science.gov (United States)

Scuderi, V.; Milluzzo, G.; Alejo, A.; Amico, A. G.; Booth, N.; Cirrone, G. A. P.; Doria, D.; Green, J.; Kar, S.; Larosa, G.; Leanza, R.; Margarone, D.; McKenna, P.; Padda, H.; Petringa, G.; Pipek, J.; Romagnani, L.; Romano, F.; Schillaci, F.; Borghesi, M.; Cuttone, G.; Korn, G.

2017-03-01

Nowadays the innovative high power laser-based ion acceleration technique is one of the most interesting challenges in particle acceleration field, showing attractive characteristics for future multidisciplinary applications, including medical ones. Nevertheless, peculiarities of optically accelerated ion beams make mandatory the development of proper transport, selection and diagnostics devices in order to deliver stable and controlled ion beams for multidisciplinary applications. This is the main purpose of the ELIMAIA (ELI Multidisciplinary Applications of laser-Ion Acceleration) beamline that will be realized and installed within 2018 at the ELI-Beamlines research center in the Czech Republic, where laser driven high energy ions, up to 60 MeV/n, will be available for users. In particular, a crucial role will be played by the on-line diagnostics system, recently developed in collaboration with INFN-LNS (Italy), consisting of TOF detectors, placed along the beamline (at different detection distances) to provide online monitoring of key characteristics of delivered beams, such as energy, fluence and ion species. In this contribution an overview on the ELIMAIA available ion diagnostics will be briefly given along with the preliminary results obtained during a test performed with high energy laser-driven proton beams accelerated at the VULCAN PW-laser available at RAL facility (U.K.).

Time of Flight based diagnostics for high energy laser driven ion beams

International Nuclear Information System (INIS)

Scuderi, V.; Margarone, D.; Schillaci, F.; Milluzzo, G.; Amico, A.G.; Cirrone, G.A.P.; Larosa, G.; Leanza, R.; Petringa, G.; Pipek, J.; Romano, F.; Alejo, A.; Doria, D.; Kar, S.; Borghesi, M.; Booth, N.; Green, J.; McKenna, P.; Padda, H.; Romagnani, L.

2017-01-01

Nowadays the innovative high power laser-based ion acceleration technique is one of the most interesting challenges in particle acceleration field, showing attractive characteristics for future multidisciplinary applications, including medical ones. Nevertheless, peculiarities of optically accelerated ion beams make mandatory the development of proper transport, selection and diagnostics devices in order to deliver stable and controlled ion beams for multidisciplinary applications. This is the main purpose of the ELIMAIA (ELI Multidisciplinary Applications of laser-Ion Acceleration) beamline that will be realized and installed within 2018 at the ELI-Beamlines research center in the Czech Republic, where laser driven high energy ions, up to 60 MeV/n, will be available for users. In particular, a crucial role will be played by the on-line diagnostics system, recently developed in collaboration with INFN-LNS (Italy), consisting of TOF detectors, placed along the beamline (at different detection distances) to provide online monitoring of key characteristics of delivered beams, such as energy, fluence and ion species. In this contribution an overview on the ELIMAIA available ion diagnostics will be briefly given along with the preliminary results obtained during a test performed with high energy laser-driven proton beams accelerated at the VULCAN PW-laser available at RAL facility (U.K.).

Comparison of biomolecule desorption yields for low and high energy primary ions

International Nuclear Information System (INIS)

Kamensky, I.; Hakansson, P.; Sundqvist, B.; McNeal, C.J.; MacFarlane, R.

1982-01-01

Ion induced desorption yields of molecular ions from samples of cesium iodide, glycylglycine, ergosterol, bleomycin and a trinucleoside diphosphate have been studied using primary beams of 54 MeV 63 Cu 9+ and 3 keV 133 Cs + . Mass analysis was performed with a time-of-flight technique. Each sample was studied with the same spectrometer for both low and high energy primary ions and without opening of the vacuum chamber in between the measurements. The results show that fast heavy ions give larger yields for all samples studied and that the yield ratios for high to low energy desorption increase with the mass of the sample molecule. (orig.)

Phosphorus Sorption Capacity of Gray Forest Soil as Dependent on Fertilization System

Science.gov (United States)

Rogova, O. B.; Kolobova, N. A.; Ivanov, A. L.

2018-05-01

In this paper, the results of the study of changes in the phosphorus sorption capacity of gray forest soils of Vladimir opolie under the impact of different fertilization systems are discussed. The quantitative parameters of the potential buffer capacity of soils for phosphorus (PBCP) and Langmuir sorption isotherms have been calculated. It is shown that the application of organic fertilizers results in a stronger decrease in PBCP than the application of mineral fertilizers. The portion of phosphorus of mineral compounds considerably increases, and the high content of available phosphates is maintained. In the variants with application of mineral phosphorus in combination with manure, the portions of organic and mineral phosphorus are at the level typical of unfertilized soils. The energy of phosphate bonds with the soil is minimal upon the application of a double rate of mineral phosphorus at the maximum capacity in relation to phosphate ions.

Radiative recombination of highly charged ions: Enhanced rates at low energies

International Nuclear Information System (INIS)

Frank, A.; Mueller, A.; Haselbauer, J.; Schennach, S.; Spies, W.; Uwira, O.; Wagner, M.

1992-01-01

In a single-pass merged-beams experiment employing a dense cold electron target recombination of highly charged ions is studied. Unexpected high recombination rates are observed at low energies E cm in the electron-ion center-of-mass frame. In particular, theoretical estimates for radiative recombination are dramatically exceeded by the experimental recombination rates at E cm =0 eV for U 28+ and for Au 25+ ions. Considerable rate enhancement is also observed for Ar 15+ . This points to a general phenomenon which has to be interpreted as a consequence of high electron densities, low electron beam temperatures, high ion charge states and presence of strong magnetic fields. (orig.)

Live cell imaging combined with high-energy single-ion microbeam

Energy Technology Data Exchange (ETDEWEB)

Guo, Na; Du, Guanghua, E-mail: gh-du@impcas.ac.cn; Liu, Wenjing; Wu, Ruqun; Wei, Junzhe [Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou (China); Guo, Jinlong [Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou (China); Northwest Normal University, Lanzhou (China); Chen, Hao [Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou (China); Institute of Nuclear Science and Technology, University of Lanzhou, Lanzhou (China)

2016-03-15

DNA strand breaks can lead to cell carcinogenesis or cell death if not repaired rapidly and efficiently. An online live cell imaging system was established at the high energy microbeam facility at the Institute of Modern Physics to study early and fast cellular response to DNA damage after high linear energy transfer ion radiation. The HT1080 cells expressing XRCC1-RFP were irradiated with single high energy nickel ions, and time-lapse images of the irradiated cells were obtained online. The live cell imaging analysis shows that strand-break repair protein XRCC1 was recruited to the ion hit position within 20 s in the cells and formed bright foci in the cell nucleus. The fast recruitment of XRCC1 at the ion hits reached a maximum at about 200 s post-irradiation and then was followed by a slower release into the nucleoplasm. The measured dual-exponential kinetics of XRCC1 protein are consistent with the proposed consecutive reaction model, and the measurements obtained that the reaction rate constant of the XRCC1 recruitment to DNA strand break is 1.2 × 10{sup −3} s{sup −1} and the reaction rate constant of the XRCC1 release from the break-XRCC1 complex is 1.2 × 10{sup −2} s{sup −1}.

Live cell imaging combined with high-energy single-ion microbeam

International Nuclear Information System (INIS)

Guo, Na; Du, Guanghua; Liu, Wenjing; Wu, Ruqun; Wei, Junzhe; Guo, Jinlong; Chen, Hao

2016-01-01

DNA strand breaks can lead to cell carcinogenesis or cell death if not repaired rapidly and efficiently. An online live cell imaging system was established at the high energy microbeam facility at the Institute of Modern Physics to study early and fast cellular response to DNA damage after high linear energy transfer ion radiation. The HT1080 cells expressing XRCC1-RFP were irradiated with single high energy nickel ions, and time-lapse images of the irradiated cells were obtained online. The live cell imaging analysis shows that strand-break repair protein XRCC1 was recruited to the ion hit position within 20 s in the cells and formed bright foci in the cell nucleus. The fast recruitment of XRCC1 at the ion hits reached a maximum at about 200 s post-irradiation and then was followed by a slower release into the nucleoplasm. The measured dual-exponential kinetics of XRCC1 protein are consistent with the proposed consecutive reaction model, and the measurements obtained that the reaction rate constant of the XRCC1 recruitment to DNA strand break is 1.2 × 10"−"3 s"−"1 and the reaction rate constant of the XRCC1 release from the break-XRCC1 complex is 1.2 × 10"−"2 s"−"1.

Recoil implantation of boron into silicon by high energy silicon ions

Science.gov (United States)

Shao, L.; Lu, X. M.; Wang, X. M.; Rusakova, I.; Mount, G.; Zhang, L. H.; Liu, J. R.; Chu, Wei-Kan

2001-07-01

A recoil implantation technique for shallow junction formation was investigated. After e-gun deposition of a B layer onto Si, 10, 50, or 500 keV Si ion beams were used to introduce surface deposited B atoms into Si by knock-on. It has been shown that recoil implantation with high energy incident ions like 500 keV produces a shallower B profile than lower energy implantation such as 10 keV and 50 keV. This is due to the fact that recoil probability at a given angle is a strong function of the energy of the primary projectile. Boron diffusion was showed to be suppressed in high energy recoil implantation and such suppression became more obvious at higher Si doses. It was suggested that vacancy rich region due to defect imbalance plays the role to suppress B diffusion. Sub-100 nm junction can be formed by this technique with the advantage of high throughput of high energy implanters.

Fifth high-energy heavy-ion study

International Nuclear Information System (INIS)

1981-10-01

This was the fifth of a continuing series of summer studies held at LBL to discuss high energy heavy ion collisions. Recently, a similar meeting has been held on alternate years at GSI (Darmstadt); and, in 1979, we held a meeting at LBL exclusively devoted to ultra-relativistic nuclear collisions. Two new features distinguish this study from earlier meetings in the series. First, the energy range for discussion was broadened by including collisions from about 20 MeV/nucleon to the highest available in the cosmic radiation. The lower range, particularly below 100 MeV/nucleon, will be under intense study in the near future with machines such as the upgraded Bevalac, Michigan State University Superconducting Cyclotron, GANIL in France, and the SC at CERN. Recently, the high energy collision regime has been expanded by the successful operation of the CERN ISR with alpha particles. Second, in addition to an extensive program of invited talks, we decided for the first time to actively solicit contributions. Forty-seven individual items from the conference were prepared separately for the data base

Fifth high-energy heavy-ion study

Energy Technology Data Exchange (ETDEWEB)

1981-10-01

This was the fifth of a continuing series of summer studies held at LBL to discuss high energy heavy ion collisions. Recently, a similar meeting has been held on alternate years at GSI (Darmstadt); and, in 1979, we held a meeting at LBL exclusively devoted to ultra-relativistic nuclear collisions. Two new features distinguish this study from earlier meetings in the series. First, the energy range for discussion was broadened by including collisions from about 20 MeV/nucleon to the highest available in the cosmic radiation. The lower range, particularly below 100 MeV/nucleon, will be under intense study in the near future with machines such as the upgraded Bevalac, Michigan State University Superconducting Cyclotron, GANIL in France, and the SC at CERN. Recently, the high energy collision regime has been expanded by the successful operation of the CERN ISR with alpha particles. Second, in addition to an extensive program of invited talks, we decided for the first time to actively solicit contributions. Forty-seven individual items from the conference were prepared separately for the data base. (GHT)

Confinement characteristics of high-energy ions produced by ICRF heating in the large helical device

International Nuclear Information System (INIS)

Kumazawa, R; Saito, K; Torii, Y; Mutoh, T; Seki, T; Watari, T; Osakabe, M; Murakami, S; Sasao, M; Watanabe, T; Yamamoto, T; Notake, T; Takeuchi, N; Saida, T; Shimpo, F; Nomura, G; Yokota, M; Kato, A; Zao, Y; Okada, H; Isobe, M; Ozaki, T; Narihara, K; Nagayama, Y; Inagaki, S; Morita, S; Krasilnikov, A V; Idei, H; Kubo, S; Ohkubo, K; Sato, M; Shimozuma, T; Yoshimura, Y; Ikeda, K; Nagaoka, K; Oka, Y; Takeiri, Y; Tsumori, K; Ashikawa, N; Emoto, M; Funaba, H; Goto, M; Ida, K; Kobuchi, T; Liang, Y; Masuzaki, S; Minami, T; Miyazawa, J; Morisaki, T; Muto, S; Nakamura, Y; Nakanishi, H; Nishimura, K; Noda, N; Ohdachi, S; Peterson, B J; Sagara, A; Sakakibara, S; Sakamoto, R; Sato, K; Shoji, M; Suzuki, H; Tanaka, K; Toi, K; Tokuzawa, T; Watanabe, K Y; Yamada, I; Yamamoto, S; Yoshinuma, M; Yokoyama, M; Watanabe, K-Y; Kaneko, O; Kawahata, K; Komori, A; Ohyabu, N; Yamada, H; Yamazaki, K; Sudo, S; Matsuoka, K; Hamada, Y; Motojima, O; Fujiwara, M

2003-01-01

The behaviour of high-energy ions accelerated by an ion cyclotron range of frequency (ICRF) electric field in the large helical device (LHD) is discussed. A better confinement performance of high-energy ions in the inward-shifted magnetic axis configuration was experimentally verified by measuring their energy spectrum and comparing it with the effective temperature determined by an electron slowing down process. In the standard magnetic axis configuration a saturation of the measured tail temperature was observed as the effective temperature was increased. The ratio between these two quantities is a measure of the quality of transfer efficiency from high-energy ions to a bulk plasma; when this efficiency was compared with Monte Carlo simulations the results agreed fairly well. The ratio of the stored energy of the high-energy ions to that of the bulk plasma was measured using an ICRF heating power modulation method; it was deduced from phase differences between total and bulk plasma stored energies and the modulated ICRF heating power. The measured high energy fraction agreed with that calculated using the injected ICRF heating power, the transfer efficiency determined in the experiment and the confinement scaling of the LHD plasma

Study of high energy ion loss during hydrogen minority heating in TFTR

International Nuclear Information System (INIS)

Park, J.; Zweben, S.J.

1994-03-01

High energy ion loss during hydrogen minority ICRF heating is measured and compared with the loss of the D-D fusion products. During H minority heating a relatively large loss of high energy ions is observed at 45 degrees below the outer midplane, with or without simultaneous NBI heating. This increase is most likely due to a loss of the minority tail protons, a possible model for this process is described

High energy structures in heavy ion collisions: a multiphonon description

International Nuclear Information System (INIS)

Chomaz, P.; Blumenfeld, Y.; Frascaria, N.

1984-01-01

Energy spectra of fragments from the 36 Ar + 208 Pb reaction at 11 MeV/n exhibit structures at high excitation energies. These structures are interpreted in terms of target multi-phonon excitations built from giant resonances. The importance of such processes for the kinetic energy dissipation in heavy ion collisions is emphasized

High energy ion microbeams and their applications

International Nuclear Information System (INIS)

Bakhru, H.; Nickles, E.; Haberl, A.; Morris, W.G.

1992-01-01

In recent years there has been rapid growth for the development of equipment for forming a focussed beam (0.5 - 2μm) with high energy ions. The State University of New York at Albany ion scanning microprobe has been used for several applications especially in the fields of materials and biological studies. Rutherford backscattering spectroscopy (RBS) and particle-induced x-ray emission (PIXE) analysis have been performed on microelectronic circuits with a spatial resolution of approximately 2 μm. Studies on films of superconductors (YBa CuO) will be presented. Applications of microbeams for the biological studies and analytical techniques will be presented. Current and future role of microbeams and their limitations will be discussed. (author)

Photon and dilepton production in high-energy heavy-ion collisions

Indian Academy of Sciences (India)

2015-05-07

May 7, 2015 ... The recent results on direct photons and dileptons in high-energy heavy-ion collisions, obtained particularly at Relativistic Heavy Ion Collider (RHIC) and Large Hadron Collider (LHC) are reviewed. The results are new not only in terms of the probes, but also in terms of the precision. We shall discuss the ...

Radiation induced phosphorus segregation in austenitic and ferritic alloys

International Nuclear Information System (INIS)

Brimhall, J.L.; Baer, D.R.; Jones, R.H.

1984-01-01

The radiation induced surface segregation (RIS) of phosphorus in stainless steel attained a maximum at a dose of 0.8 dpa then decreased continually with dose. This decrease in the surface segregation of phosphorus at high dose levels has been attributed to removal of the phosphorus layer by ion sputtering. Phosphorus is not replenished since essentially all of the phosphorus within the irradiation zone has been segregated to the surface. Sputter removal can explain the previously reported absence of phosphorus segregation in ferritic alloys irradiated at high dosessup(1,2) (>1 dpa) since irradiation of ferritic alloys to low doses has shown measurable RIS. This sputtering phenomenon places an inherent limitation to the heavy ion irradiation technique for the study of surface segregation of impurity elements. The magnitude of the segregation in ferritics is still much less than in stainless steel which can be related to the low damage accumulation in these alloys. (orig.)

A model for high-energy heavy-ion collisions

International Nuclear Information System (INIS)

Myers, W.D.

1978-01-01

A model is developed for high-energy heavy-ion collisions that treats the variation across the overlap region of the target and projectile in the amount of energy and momentum that is deposited. The expression for calculating any observable takes the form of a sum over a series of terms, each one of which consists of a geometric, a kinematic, and a statistical factor. The geometrical factors for a number of target projectile systems are tabulated. (Auth.)

Heavy ion reactions at high energies

International Nuclear Information System (INIS)

Jakobsson, Bo.

1977-01-01

A review on heavy ion experiments at energies >0.1GeV/nucleon is presented. Reaction cross-sections, isotope production cross-sections and pion production in nucleus-nucleus collisions are discussed. Some recent models for heavy ion reactions like the abrasion-ablation model, the fireball model and the different shock-wave models are also presented

Highly Oriented Graphene Sponge Electrode for Ultra High Energy Density Lithium Ion Hybrid Capacitors.

Science.gov (United States)

Ahn, Wook; Lee, Dong Un; Li, Ge; Feng, Kun; Wang, Xiaolei; Yu, Aiping; Lui, Gregory; Chen, Zhongwei

2016-09-28

Highly oriented rGO sponge (HOG) can be easily synthesized as an effective anode for application in high-capacity lithium ion hybrid capacitors. X-ray diffraction and morphological analyses show that successfully exfoliated rGO sponge on average consists of 4.2 graphene sheets, maintaining its three-dimensional structure with highly oriented morphology even after the thermal reduction procedure. Lithium-ion hybrid capacitors (LIC) are fabricated in this study based on a unique cell configuration which completely eliminates the predoping process of lithium ions. The full-cell LIC consisting of AC/HOG-Li configuration has resulted in remarkably high energy densities of 231.7 and 131.9 Wh kg(-1) obtained at 57 W kg(-1) and 2.8 kW kg(-1). This excellent performance is attributed to the lithium ion diffusivity related to the intercalation reaction of AC/HOG-Li which is 3.6 times higher that of AC/CG-Li. This unique cell design and configuration of LIC presented in this study using HOG as an effective anode is an unprecedented example of performance enhancement and improved energy density of LIC through successful increase in cell operation voltage window.

Martensitic transformation of type 304 stainless steel by high-energy ion implantation

International Nuclear Information System (INIS)

Chayahara, A.; Satou, M.; Nakashima, S.; Hashimoto, M.; Sasaki, T.; Kurokawa, M.; Kiyama, S.

1991-01-01

The effect of high-energy ion implantation on the structural changes of type 304 stainless steel were investigated. Gold, copper and silicon ions with an energy of 1.5 MeV was implanted into stainless steel. The fluences were in the range from 5x10 15 to 10 17 ions/cm 2 . It was found that the structure of stainless steel was transformed form the austenitic to the martensitic structure by these ion implantations. This structural change was investigated by means of X-ray diffraction and transmission electron microscopy (TEM). The depth profile of the irradiated ions was also analyzed by secondary ion mass spectroscopy (SIMS) and glow discharge spectroscopy (GDS). The degree of martensitic transformation was found to be strongly dependent on the surface pretreatment, either mechanical or electrolytic polishing. When the surface damages or strains by mechanical polishing were present, the martensitic transformation was greatly accelerated presumably due to the combined action of ion irradiation and strain-enhanced transformation. Heavier ions exhibit a high efficiency for the transformation. (orig.)

New improvements on the Kansas State University cryogenic electron beam ion source, a user facility for low energy, highly charged ions

International Nuclear Information System (INIS)

Stockli, M. P.; Carnes, K.; Cocke, C. L.; DePaola, B. D.; Ehrenreich, T.; Fehrenbach, C.; Fry, D.; Gibson, P. E.; Kelly, S.; Lehnert, U.

2000-01-01

The Kansas State University cryogenic electron beam ion source supplies low energy ion beams to users of the Department of Energy user facility for highly charged ions. The ions escape the source with an initial energy between 1.6 and 5 kV per charge and are analyzed in a 90 degree sign dipole magnet located on the high voltage platform. When leaving the platform the ions can be accelerated by up to 160 kV per charge or can be decelerated to about 20% of their initial energy, covering 2.5 orders of magnitude. We are in the process of adding another order of magnitude to the range of available ion energies as a newly installed lens allows for deceleration down to a very few percent of the initial energy. In addition we present the current microbunching and chopping system which has been substantially improved over the past 2 yr. (c) 2000 American Institute of Physics

Escape of high-energy oxygen ions through magnetopause reconnection under northward IMF

Directory of Open Access Journals (Sweden)

S. Kasahara

2008-12-01

Full Text Available During a storm recovery phase on 15 May 2005, the Geotail spacecraft repeatedly observed high-energy (>180 keV oxygen ions in the dayside magnetosheath near the equatorial plane. We focused on the time period from 11:20 UT to 13:00 UT, when Geotail observed the oxygen ions and the interplanetary magnetic field (IMF was constantly northward. The magnetic reconnection occurrence northward and duskward of Geotail is indicated by the Walén analysis and convective flows in the magnetopause boundary layer. Anisotropic pitch angle distributions of ions suggest that high-energy oxygen ions escaped from the northward of Geotail along the reconnected magnetic field lines. From the low-energy particle precipitation in the polar cap observed by DMSP, which is consistent with magnetic reconnection occurring between the magnetosheath field lines and the magnetospheric closed field lines, we conclude that these oxygen ions are of ring current origin. Our results thus suggest a new escape route of oxygen ions during northward IMF. In the present event, this escape mechanism is more dominant than the leakage via the finite Larmor radius effect across the dayside equatorial magnetopause.

The influence of excess vacancy generation on the diffusion of ion implanted phosphorus into silicon

International Nuclear Information System (INIS)

Bakowski, A.

1985-01-01

The diffusion of ion implanted phosphorus in silicon has been studied. It was found that the diffusion coefficient is not only dependent on the phosphorus surface concentration (the concentration effect) but also on the conditions at the silicon surface (the surface effect). The phosphorus diffusion coefficient is considerably lower when the silicon surface during annealing is covered with a CVD oxide layer. It is suggested that excess vacancies generated at the surface are reponsible for both the concentration and surface effects. Enhanced phosphorus diffusion is attributed to the disturbance of thermodynamic equilibrium in the crystal through phosphorus-vacancy part formation by vacancies introduced into silicon at the surface. On the basis of the data presented, it can be concluded that two mechanisms for excess vacancy generation are involved. Assuming that phosphorus diffuses via E-centers, calculations of the concentration profiles and the diffusion coefficient were performed for different concentrations and surface conditions. (orig.)

Simulating antler growth and energy, nitrogen, calcium and phosphorus metabolism in caribou

Directory of Open Access Journals (Sweden)

Ron Moen

1998-03-01

Full Text Available We added antler growth and mineral metabolism modules to a previously developed energetics model for ruminants to simulate energy and mineral balance of male and female caribou throughout an annual cycle. Body watet, fat, protein, and ash are monitored on a daily time step, and energy costs associated with reproduction and body mass changes are simulated. In order to simulate antler growth, we had to predict calcium and phosphorus metabolism as it is affected by antler growth, gestation, and lactation. We used data on dietary digestibility, protein, calcium and phosphorus content, and seasonal patterns in body mass to predict the energy, nitrogen, calcium, and phosphorus balances of a "generic" male and female caribou. Antler growth in males increased energy requirements during antler growth by 8 to 16%, depending on the efficiency with which energy was used for antler growth. Female energy requirements for antler growth were proportionately much smaller because of the smaller size of female antlers. Protein requirements for antler growth in both males and females were met by forage intake. Calcium and phosphorus must be resorbed from bone during peak antler growth in males, when > 25 g/day of calcium and > 12 g/day of phosphorus are being deposited in antlers. Females are capable of meeting calcium needs during antler growth without bone resorption, but phosphorus was resorbed from bone during the final stages of antler mineralization. After energy, phosphorus was most likely to limit growth of antlers for both males and females in our simulations. Input parameters can be easily changed to represent caribou from specific geographic regions in which dietary nutrient content or body mass patterns differ from those in our "generic" caribou. The model can be used to quantitatively analyze the evolutionary basis for development of antlers in female caribou, and the relationship between body mass and antler size in the Cervidae.

Recent US advances in ion-beam-driven high energy density physics and heavy ion fusion

International Nuclear Information System (INIS)

Logan, B.G.; Bieniosek, F.M.; Celata, C.M.; Coleman, J.; Greenway, W.; Henestroza, E.; Kwan, J.W.; Lee, E.P.; Leitner, M.; Roy, P.K.; Seidl, P.A.; Vay, J.-L.; Waldron, W.L.; Yu, S.S.; Barnard, J.J.; Cohen, R.H.; Friedman, A.; Grote, D.P.; Kireeff Covo, M.; Molvik, A.W.; Lund, S.M.; Meier, W.R.; Sharp, W.; Davidson, R.C.; Efthimion, P.C.; Gilson, E.P.; Grisham, L.; Kaganovich, I.D.; Qin, H.; Sefkow, A.B.; Startsev, E.A.; Welch, D.; Olson, C.

2007-01-01

During the past two years, significant experimental and theoretical progress has been made in the US heavy ion fusion science program in longitudinal beam compression, ion-beam-driven warm dense matter, beam acceleration, high brightness beam transport, and advanced theory and numerical simulations. Innovations in longitudinal compression of intense ion beams by >50X propagating through background plasma enable initial beam target experiments in warm dense matter to begin within the next two years. We are assessing how these new techniques might apply to heavy ion fusion drivers for inertial fusion energy

Review of high energy heavy ion experiments

International Nuclear Information System (INIS)

Miake, Yasuo

2000-01-01

It has been proposed that in high energy heavy ion collisions a physical conditions similar to the early stage of the Universe can be established in the laboratory. New phase of matter expected to be created is called the quark gluon plasma (QGP). Based on the motivation to create the QGP in the laboratory, heavy ion beams have been accelerated at AGS of Brookhaven National Laboratory and also at CERN-SPS. Several interesting features of the data have been reported, among which are: the suppression of J/ψ production in Pb+Pb collisions, the enhancement of low mass lepton pairs, and the collective behavior of hadron production. These features are reviewed under the key words of Deconfinement, Chiral Restoration and Collectivity in the lecture. (author)

High energy density in matter produced by heavy ion beams

International Nuclear Information System (INIS)

1987-08-01

This annual report summarizes the results of research carried out in 1986 within the framework of the program 'High Energy Density in Matter Produced by Heavy Ion Beams' which is funded by the Federal Ministry for Research and Technology. Its initial motivation and its ultimate goal is the question whether inertial confinement can be achieved by intense beams of heavy ions. (orig./HSI)

Achieving High-Energy-High-Power Density in a Flexible Quasi-Solid-State Sodium Ion Capacitor.

Science.gov (United States)

Li, Hongsen; Peng, Lele; Zhu, Yue; Zhang, Xiaogang; Yu, Guihua

2016-09-14

Simultaneous integration of high-energy output with high-power delivery is a major challenge for electrochemical energy storage systems, limiting dual fine attributes on a device. We introduce a quasi-solid-state sodium ion capacitor (NIC) based on a battery type urchin-like Na2Ti3O7 anode and a capacitor type peanut shell derived carbon cathode, using a sodium ion conducting gel polymer as electrolyte, achieving high-energy-high-power characteristics in solid state. Energy densities can reach 111.2 Wh kg(-1) at power density of 800 W kg(-1), and 33.2 Wh kg(-1) at power density of 11200 W kg(-1), which are among the best reported state-of-the-art NICs. The designed device also exhibits long-term cycling stability over 3000 cycles with capacity retention ∼86%. Furthermore, we demonstrate the assembly of a highly flexible quasi-solid-state NIC and it shows no obvious capacity loss under different bending conditions.

Silicon-Based Lithium-Ion Capacitor for High Energy and High Power Application

Science.gov (United States)

Wu, James J.; Demattia, Brianne; Loyselle, Patricia; Reid, Concha; Kohout, Lisa

2017-01-01

Si-based Li-ion capacitor has been developed and demonstrated. The results show it is feasible to improve both power density and energy density in this configuration. The applied current density impacts the power and energy density: low current favors energy density while high current favors power density. Active carbon has a better rate capability than Si. Next StepsFuture Directions. Si electrode needs to be further studied and improved. Further optimization of SiAC ratio and evaluation of its impact on energy density and power density.

A Quasi-Solid-State Sodium-Ion Capacitor with High Energy Density.

Science.gov (United States)

Wang, Faxing; Wang, Xiaowei; Chang, Zheng; Wu, Xiongwei; Liu, Xiang; Fu, Lijun; Zhu, Yusong; Wu, Yuping; Huang, Wei

2015-11-18

A quasi-solid-state sodium-ion capacitor is demonstrated with nanoporous disordered carbon and macroporous graphene as the negative and positive electrodes, respectively, using a sodium-ion-conducting gel polymer electrolyte. It can operate at a cell voltage as high as 4.2 V with an energy density of record high 168 W h kg(-1). © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Lifetimes of relativistic heavy-ion beams in the High Energy Storage Ring of FAIR

Science.gov (United States)

Shevelko, V. P.; Litvinov, Yu. A.; Stöhlker, Th.; Tolstikhina, I. Yu.

2018-04-01

The High Energy Storage Ring, HESR, will be constructed at the Facility for Antiproton and Ion Research, FAIR, Darmstadt. For the first time, it will be possible to perform experiments with cooled high-intensity stable and radioactive heavy ions at highly relativistic energies. To design experiments at the HESR, realistic estimations of beam lifetimes are indispensable. Here we report calculated cross sections and lifetimes for typical U88+ , U90+ , U92+ , Sn49+ and Sn50+ ions in the energy range E = 400 MeV/u-5 GeV/u, relevant for the HESR. Interactions with the residual gas and with internal gas-jet targets are also considered.

Formation of the high-energy ion population in the earth's magnetotail: spacecraft observations and theoretical models

Directory of Open Access Journals (Sweden)

A. V. Artemyev

2014-10-01

Full Text Available We investigate the formation of the high-energy (E ∈ [20,600] keV ion population in the earth's magnetotail. We collect statistics of 4 years of Interball / Tail observations (1995–1998 in the vicinity of the neutral plane in the magnetotail region (X RE, |Y| ≤ 20 RE in geocentric solar magnetospheric (GSM system. We study the dependence of high-energy ion spectra on the thermal-plasma parameters (the temperature Ti and the amplitude of bulk velocity vi and on the magnetic-field component Bz. The ion population in the energy range E ∈ [20,600] keV can be separated in the thermal core and the power-law tail with the slope (index ~ −4.5. Fluxes of the high-energy ion population increase with the growth of Bz, vi and especially Ti, but spectrum index seems to be independent on these parameters. We have suggested that the high-energy ion population is generated by small scale transient processes, rather than by the global reconfiguration of the magnetotail. We have proposed the relatively simple and general model of ion acceleration by transient bursts of the electric field. This model describes the power-law energy spectra and predicts typical energies of accelerated ions.

U.S. Heavy Ion Beam Research for High Energy Density Physics Applications and Fusion

International Nuclear Information System (INIS)

Davidson, R.C.; Logan, B.G.; Barnard, J.J.; Bieniosek, F.M.; Briggs, R.J.

2005-01-01

Key scientific results from recent experiments, modeling tools, and heavy ion accelerator research are summarized that explore ways to investigate the properties of high energy density matter in heavy-ion-driven targets, in particular, strongly-coupled plasmas at 0.01 to 0.1 times solid density for studies of warm dense matter, which is a frontier area in high energy density physics. Pursuit of these near-term objectives has resulted in many innovations that will ultimately benefit heavy ion inertial fusion energy. These include: neutralized ion beam compression and focusing, which hold the promise of greatly improving the stage between the accelerator and the target chamber in a fusion power plant; and the Pulse Line Ion Accelerator (PLIA), which may lead to compact, low-cost modular linac drivers

Confinement improvement in high-ion temperature plasmas heated with high-energy negative-NBI in LHD

International Nuclear Information System (INIS)

Takeiri, Y.; Morita, S.; Ikeda, K.

2006-10-01

The increase in the ion temperature due to transport improvement has been observed in plasmas heated with high-energy negative-NBI, in which electrons are dominantly heated, in Large Helical Device (LHD). When the centrally focused ECRH is superposed on the NBI plasma, the ion temperature is observed to rise, accompanied by formation of the electron-ITB. This is ascribed to the ion transport improvement with the transition to the neoclassical electron root with a positive radial electric field. In high-Z plasmas, the ion temperature is increased with an increase in the ion heating power, and reaches 13.5keV. The central ion temperature increases with an increase in a gradient of the electron temperature in an outer plasma region of ρ=0.8, suggesting the ion transport improvement in the outer plasma region induced by the neoclassical electron root. These results indicate the effectiveness of the electron-root scenario for obtaining high-ion temperature plasmas in helical systems. (author)

ECR ion source based low energy ion beam facility

Indian Academy of Sciences (India)

Mass analyzed highly charged ion beams of energy ranging from a few keV to a few MeV plays an important role in various aspects of research in modern physics. In this paper a unique low energy ion beam facility (LEIBF) set up at Nuclear Science Centre (NSC) for providing low and medium energy multiply charged ion ...

High-energy heavy ion testing of VLSI devices for single event ...

Indian Academy of Sciences (India)

Unknown

per describes the high-energy heavy ion radiation testing of VLSI devices for single event upset (SEU) ... The experimental set up employed to produce low flux of heavy ions viz. silicon ... through which they pass, leaving behind a wake of elec- ... for use in Bus Management Unit (BMU) and bulk CMOS ... was scheduled.

Flexible Aqueous Li-Ion Battery with High Energy and Power Densities.

Science.gov (United States)

Yang, Chongyin; Ji, Xiao; Fan, Xiulin; Gao, Tao; Suo, Liumin; Wang, Fei; Sun, Wei; Chen, Ji; Chen, Long; Han, Fudong; Miao, Ling; Xu, Kang; Gerasopoulos, Konstantinos; Wang, Chunsheng

2017-11-01

A flexible and wearable aqueous symmetrical lithium-ion battery is developed using a single LiVPO 4 F material as both cathode and anode in a "water-in-salt" gel polymer electrolyte. The symmetric lithium-ion chemistry exhibits high energy and power density and long cycle life, due to the formation of a robust solid electrolyte interphase consisting of Li 2 CO 3 -LiF, which enables fast Li-ion transport. Energy densities of 141 Wh kg -1 , power densities of 20 600 W kg -1 , and output voltage of 2.4 V can be delivered during >4000 cycles, which is far superior to reported aqueous energy storage devices at the same power level. Moreover, the full cell shows unprecedented tolerance to mechanical stress such as bending and cutting, where it not only does not catastrophically fail, as most nonaqueous cells would, but also maintains cell performance and continues to operate in ambient environment, a unique feature apparently derived from the high stability of the "water-in-salt" gel polymer electrolyte. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Nuclear interactions in high energy heavy ions and applications in astrophysics

International Nuclear Information System (INIS)

Wefel, J.P.; Guzik, T.G.

1993-01-01

The overall objective is to study the mechanisms and the energy dependence of heavy ion fragmentation by studying the reactions of heavy ion projectiles (e.g. 4 He, 16 O, 20 Ne, 28 Si, 56 Fe) in a variety of targets (H, He, C, Si, Cu, Pb) and at a number of beam energies exceeding 0.1 GeV/nucleon. The results have application to questions in high-energy nuclear astrophysics. Most of the discussion is on low-energy 16 O, 28 Si data analysis. The description includes analysis procedures and techniques, detector calibrations, data selections and normalizations. Cross section results for the analysis are also presented. 83 figs., 6 tabs., 73 refs

Highly efficient generation of ultraintense high-energy ion beams using laser-induced cavity pressure acceleration

Energy Technology Data Exchange (ETDEWEB)

Badziak, J.; Jablonski, S.; Raczka, P. [Institute of Plasma Physics and Laser Microfusion, Euratom Association, 01-497 Warsaw (Poland)

2012-08-20

Results of particle-in-cell (PIC) simulations of fast ion generation in the recently proposed laser-induced cavity pressure acceleration (LICPA) scheme in which a picosecond circularly polarized laser pulse of intensity {approx}10{sup 21} W/cm{sup 2} irradiates a carbon target placed in a cavity are presented. It is shown that due to circulation of the laser pulse in the cavity, the laser-ions energy conversion efficiency in the LICPA scheme is more than twice as high as that for the conventional (without a cavity) radiation pressure acceleration scheme and a quasi-monoenergetic carbon ion beam of the mean ion energy {approx}0.5 GeV and the energy fluence {approx}0.5 GJ/cm{sup 2} is produced with the efficiency {approx}40%. The results of PIC simulations are found to be in fairly good agreement with the predictions of the generalized light-sail model.

Photon and dilepton production in high-energy heavy-ion collisions

Indian Academy of Sciences (India)

2015-05-07

May 7, 2015 ... Photons; dileptons; Relativistic Heavy Ion Collider; Large Hadron Collider; quark ... the collisions produces relatively high pT photons, often referred to ..... energy have been found for identified charged hadrons at RHIC [25].

Ge nano-layer fabricated by high-fluence low-energy ion implantation

International Nuclear Information System (INIS)

Lu Tiecheng; Dun Shaobo; Hu Qiang; Zhang Songbao; An Zhu; Duan Yanmin; Zhu Sha; Wei Qiangmin; Wang Lumin

2006-01-01

A Ge nano-layer embedded in the surface layer of an amorphous SiO 2 film was fabricated by high-fluence low-energy ion implantation. The component, phase, nano-structure and luminescence properties of the nano-layer were studied by means of Rutherford backscattering, glancing incident X-ray diffraction, laser Raman scattering, transmission electron microscopy and photoluminescence. The relation between nano-particle characteristics and ion fluence was also studied. The results indicate that nano-crystalline Ge and nano-amorphous Ge particles coexist in the nano-layer and the ratio of nano-crystalline Ge to nano-particle Ge increases with increasing ion fluence. The intensity of photoluminescence from the nano-layer increases with increasing ion fluence also. Prepared with certain ion fluences, high-density nano-layers composed of uniform-sized nano-particles can be observed

Medium energy ion scattering (MEIS)

International Nuclear Information System (INIS)

Dittmann, K.; Markwitz, A.

2009-01-01

This report gives an overview about the technique and experimental study of medium energy ion scattering (MEIS) as a quantitative technique to determine and analyse the composition and geometrical structure of crystalline surfaces and near surface-layers by measuring the energy and yield of the backscattered ions. The use of a lower energy range of 50 to 500 keV accelerated ions impinging onto the target surface and the application of a high-resolution electrostatic energy analyser (ESA) makes medium energy ion scattering spectroscopy into a high depth resolution and surface-sensitive version of RBS with less resulting damage effects. This report details the first steps of research in that field of measurement technology using medium energetic backscattered ions detected by means of a semiconductor radiation detector instead of an ESA. The study of medium energy ion scattering (MEIS) has been performed using the 40 keV industrial ion implanter established at GNS Sciences remodelled with supplementary high voltage insulation for the ion source in order to apply voltages up to 45 kV, extra apertures installed in the beamline and sample chamber in order to set the beam diameter accurately, and a semiconductor radiation detector. For measurement purposes a beam of positive charged helium ions accelerated to an energy of about 80 keV has been used impinging onto target surfaces of lead implanted into silicon (PbSi), scandium implanted into aluminium (ScAl), aluminium foil (Al) and glassy carbon (C). First results show that it is possible to use the upgraded industrial implanter for medium energy ion scattering. The beam of 4 He 2+ with an energy up to 88 keV has been focussed to 1 mm in diameter. The 5 nA ion beam hit the samples under 2 x 10 -8 mbar. The results using the surface barrier detector show scattering events from the samples. Cooling of the detector to liquid nitrogen temperatures reduced the electronic noise in the backscattering spectrum close to zero. A

PHELIX - Petawatt high-energy laser for heavy ion experiments

International Nuclear Information System (INIS)

Backe, H.; Bock, R.; Caird, J.

1998-12-01

A high-power laser facility will be installed at the GSI heavy-ion accelerator. It will deliver laser pulses up to one kilojoule (with an option of a later upgrade to several kJ) at a pulse length of 1 - 10 nanoseconds (high-energy mode). In a high-intensity mode, laser pulses with a power of one petawatt (10 15 Watt) will be generated by chirped pulse amplification at a pulse length of typically 500 femtoseconds. Details of the laser system as well as time schedule and costs are given in Section B. In combination with the heavy-ion beams available at GSI - which will be further improved in intensity by the presently on-going upgrade program - a large number of unique experiments will become possible by the high-power laser facility described in this report. As outlined in Section A, novel research opportunities are expected in a wide range of basic-research topics spanning from the study of ion-matter interaction, through challenging new experiments in atomic, nuclear, and astrophysics, into the virgin field of relativistic plasma physics. Foreseeable topics in applied science are the development of new sources for highly charged ions and of X-ray lasers, new concepts for laser-based particle acceleration and the research in the field of inertial confinement fusion. (orig.)

Collective processes in a tokamak with high-energy particles: general problems of the linear theory of Alfven instabilities of a tokamak with high-energy ions

International Nuclear Information System (INIS)

Mikhailovskii, A.B.

1986-01-01

Some general problems of the theory of Alfven instabilities of a tokamak with high-energy ions are considered. It is assumed that such ions are due to either ionization of fast neutral atoms, injected into the tokamak, or production of them under thermo-nuclear conditions. Small-oscillation equations are derived for the Alfven-type waves, which allow for both destabilizing effects, associated with the high-energy particles, and stabilizing ones, such as effects of shear and bulk-plasm dissipation. A high-energy ion contribution is calculated into the growth rate of the Alfven waves. The author considers the role of trapped-electron collisional dissipation

Determination of phosphorus in gold or silver brazing alloys

International Nuclear Information System (INIS)

Antepenko, R.J.

1976-01-01

A spectrophotometric method has been devised for measuring microgram levels of phosphorus in brazing alloys of gold or silver alloys is normally measured by solid mass spectrometry, but the high nickel concentration produces a double ionized nickel spectral interference. The described procedures is based upon the formation of molybdovandophosphoric acid when a molybdate solution is added to an acidic solution containing orthophosphate and vanadate ions. The optimum acidity for forming the yellow colored product is 0.5 N hydrochloric acid. The working concentration range is from 0.1 to 1 ppm phosphorus using 100-mm cells and measuring the absorbance at 460 nm. The sample preparation procedure employs aqua regia to dissolve the alloy oxidize the phosphorus to orthophosphate. Cation-exchange chromatography is used to remove nickel ions and anion-exchange and chromatography to remove gold ions as the chloride complex. Excellent recoveries are obtained for standard phosphorus solutions run through the sample procedure. The procedure is applicable to a variety of gold or silver braze alloys requiring phosphorus analysis

Fine Structure Intervals ‎ ‎-‎ ‎ , ‎ ‎-‎ ‎ and ‎Electric Dipole Transition Rate ‎ ‎-‎ ‎ in ‎Phosphorus Isoelectronic Sequence ‎ ‎ ‎And Phosphorus Ions

Directory of Open Access Journals (Sweden)

Adnan Yousif Hussein

2017-11-01

Full Text Available A systematic study for the calculation of the fine structure intervals -  and -   for the ground configuration 3s23p3 and the excited configuration 3s23p24s respectively, and electric dipole transition rate -  as well as transition energy form the excited configuration 3s23p24s to the ground configuration 3s23p3 in Phosphorus isoelectronic sequence by applying multi-configuration Dirac-Fock (MCDF method. The effect of Breit interaction, QED and correlation on the fine structure interval and the gauge invariance effect on the transition probability are studied. Also the fine structure intervals for the phosphorus ions from Piii to Pxv are calculated and are compared with the available experimental data and gives good consistent

The interactions of high-energy, highly charged Xe ions with buckyballs

International Nuclear Information System (INIS)

Ali, R.; Berry, H.G.; Cheng, S.

1994-01-01

Ionization and fragmentation have been measured for C 60 molecules bombarded by highly charged (up to 35+) xenon ions with energies ranging up to 625 MeV. The observed mass distribution of positively charged fragments is explained in terms of a theoretical model indicating that the total interaction cross section contains roughly equal contributions from (a) excitation of the giant plasmon resonance, and (b) large-energy-transfer processes that lead to multiple fragmentation of the molecule. Preliminary results of measurements on VUV photons emitted in these interactions are also presented

A Hierarchical Phosphorus Nanobarbed Nanowire Hybrid: Its Structure and Electrochemical Properties.

Science.gov (United States)

Zhao, Dan; Li, Beibei; Zhang, Jinying; Li, Xin; Xiao, Dingbin; Fu, Chengcheng; Zhang, Lihui; Li, Zhihui; Li, Jun; Cao, Daxian; Niu, Chunming

2017-06-14

Nanostructured phosphorus-carbon composites are promising materials for Li-ion and Na-ion battery anodes. A hierarchical phosphorus hybrid, SiC@graphene@P, has been synthesized by the chemical vapor deposition of phosphorus on the surfaces of barbed nanowires, where the barbs are vertically grown graphene nanosheets and the cores are SiC nanowires. A temperature-gradient vaporization-condensation method has been used to remove the unhybridized phosphorus particles formed by homogeneous nucleation. The vertically grown barb shaped graphene nanosheets and a high concentration of edge carbon atoms induced a fibrous red phosphorus (f-RP) growth with its {001} planes in parallel to {002} planes of nanographene sheets and led to a strong interpenetrated interface interaction between phosphorus and the surfaces of graphene nanosheets. This hybridization has been demonstrated to significantly enhance the electrochemical performances of phosphorus.

Brookhaven four-stage accel-decel production of low-energy highly stripped heavy ions

International Nuclear Information System (INIS)

Barrette, J.; Thieberger, P.

1981-01-01

The dual MP tandem facility at Brookhaven has been used in a four-stage accel-decel mode to produce highly stripped S ion beams (Q = 10-16 + ). Fully stripped S ions were obtained at energies down to 8 MeV. The low energy limit is presently due to the inclined field configuration of the last acceleration tube

High-energy-ion depletion in the charge exchange spectrum of Alcator C

International Nuclear Information System (INIS)

Schissel, D.P.

1982-01-01

A three-dimensional, guiding center, Monte Carlo code is developed to study ion orbits in Alcator C. The highly peaked ripple of the magnetic field of Alcator is represented by an analytical expression for the vector potential. The analytical ripple field is compared to the resulting magnetic field generated by a current model of the toroidal plates; agreement is excellent. Ion-Ion scattering is simulated by a pitch angle and an energy scattering operator. The equations of motion are integrated with a variable time step, extrapolating integrator. The code produces collisionless banana and ripple trapped loss cones which agree well with present theory. Global energy distributions have been calculated and show a slight depletion above 8.5 keV. Particles which are ripple trapped and lost are at energies below where depletion is observed. It is found that ions pitch angle scatter less as energy is increased. The result is that, when viewed in velocity space, ions form probability lobes the shape of mouse ears which are fat near the thermal energy. Therefore, particles enter the loss cone at low energies near the bottom of the core. Recommendations for future work include improving the analytic model of the ripple field, testing the effect of del . B not equal to 0 on ion orbits, and improving the efficiency of the code by either using a spline fit for the magnetic fields or by creating a vectorized Monte Carlo code

Effects of high-energy (MeV) ion implantation of polyester films

International Nuclear Information System (INIS)

Ueno, Keiji; Matsumoto, Yasuyo; Nishimiya, Nobuyuki; Noshiro, Mitsuru; Satou, Mamoru

1991-01-01

The effects of high-energy ion beam irradiation on polyester (PET) films using a 3 MeV tandem-type ion beam accelerator were studied. O, Ni, Pt, and Au as ion species were irradiated at 10 14 -10 15 ions/cm 2 on 50 μm thick PET films. Physical properties and molecular structure changes were studied by the surface resistivity measurements and RBS. The surface resistivity decreases with an increase in irradiation dose. At 10 15 ions/cm 2 irradiation, the surface resistivity is 10 8 Ω/□. According to RBS and XPS analyses, some carbon and oxygen atoms in the PET are replaced by implanted ions and the -C=O bonds are destroyed easily by the ion beam. (orig.)

Phosphorus oxide gate dielectric for black phosphorus field effect transistors

Science.gov (United States)

Dickerson, W.; Tayari, V.; Fakih, I.; Korinek, A.; Caporali, M.; Serrano-Ruiz, M.; Peruzzini, M.; Heun, S.; Botton, G. A.; Szkopek, T.

2018-04-01

The environmental stability of the layered semiconductor black phosphorus (bP) remains a challenge. Passivation of the bP surface with phosphorus oxide, POx, grown by a reactive ion etch with oxygen plasma is known to improve photoluminescence efficiency of exfoliated bP flakes. We apply phosphorus oxide passivation in the fabrication of bP field effect transistors using a gate stack consisting of a POx layer grown by reactive ion etching followed by atomic layer deposition of Al2O3. We observe room temperature top-gate mobilities of 115 cm2 V-1 s-1 in ambient conditions, which we attribute to the low defect density of the bP/POx interface.

High-energy acceleration of an intense negative ion beam

International Nuclear Information System (INIS)

Takeiri, Y.; Ando, A.; Kaneko, O.

1995-02-01

A high-current H - ion beam has been accelerated with the two-stage acceleration. A large negative hydrogen ion source with an external magnetic filter produces more than 10 A of the H - ions from the grid area of 25cm x 50cm with the arc efficiency of 0.1 A/kW by seeding a small amount of cesium. The H - ion current increases according to the 3/2-power of the total beam energy. A 13.6 A of H - ion beam has been accelerated to 125 keV at the operational gas pressure of 3.4 mTorr. The optimum beam acceleration is achieved with nearly the same electric fields in the first and the second acceleration gaps on condition that the ratio of the first acceleration to the extraction electric fields is adjusted for an aspect ratio of the extraction gap. The ratio of the acceleration drain current to the H - ion current is more than 1.7. That is mainly due to the secondary electron generated by the incident H - ions on the extraction grid and the electron suppression grid. The neutralization efficiency was measured and agrees with the theoretical calculation result. (author)

Protein, energy and phosphorus supplementation of cattle fed low ...

African Journals Online (AJOL)

The effect of protein, energy and phosphorus supplements, fed ..... The results of this experiment confirm the basic concepts that ... article. The lack of response or even negative reaction to energy supplements under these conditions can be ...

Charge exchange processes of high energy heavy ions channeled in crystals

International Nuclear Information System (INIS)

Andriamonje, S.; Dural, J.; Toulemonde, M.; Groeneveld, K.O.; Maier, R.; Quere, Y.

1990-01-01

The interaction of moving ions with single crystals is very sensitive to the orientation of the incident beam with respect to the crystalline directions of the target. The experiments show that high energy heavy ion channeling deeply modifies the slowing down and charge exchange processes. In this review, we describe the opportunity offered by channeling conditions to study the charge exchange processes. Some aspects of the charge exchange processes with high energy channeled heavy ions are selected from the extensive literature published over the past few years on this subject. Special attention is given to the work performed at the GANIL facility on the study of Radiative Electron Capture (REG), Electron Impact Ionisation (EII), and convoy electron emission. Finally we emphasize the interest of studying resonant charge exchange processes such as Resonant Coherent Excitation (RCE), Resonant Transfer and Excitation (RTE) or Dielectronic Recombination (DR) and the recently proposed Nuclear Excitation by Electron Capture (NEEC)

Foldable, High Energy Density Lithium Ion Batteries

Science.gov (United States)

Suresh, Shravan

Lithium Ion Batteries (LIBs) have become ubiquitous owing to its low cost, high energy density and, power density. Due to these advantages, LIBs have garnered a lot of attention as the primary energy storage devices in consumer electronics and electric vehicles. Recent advances in the consumer electronics research and, the drive to reduce greenhouse gases have created a demand for a shape conformable, high energy density batteries. This thesis focuses on the aforementioned two aspects of LIBs: (a) shape conformability (b) energy density and provides potential solutions to enhance them. This thesis is divided into two parts viz. (i) achieving foldability in batteries and, (ii) improving its energy density. Conventional LIBs are not shape conformable due to two limitations viz. inelasticity of metallic foils, and delamination of the active materials while bending. In the first part of the thesis (in Chapter 3), this problem is solved by replacing metallic current collector with Carbon Nanotube Macrofilms (CNMs). CNMs are superelastic films comprising of porous interconnected nanotube network. Using Molecular Dynamics (MD) simulation, we found that in the presence of an interconnected nanotube network CNMs can be fully folded. This is because the resultant stress due to bending and, the effective bending angle at the interface is reduced due to the network of nanotubes. Hence, unlike an isolated nanotube (which ruptures beyond 120 degrees of bending), a network of nanotubes can be completely folded. Thus, by replacing metallic current collector foils with CNMs, the flexibility limitation of a conventional LIB can be transcended. The second part of this thesis focusses on enhancing the energy density of LIBs. Two strategies adopted to achieve this goal are (a) removing the dead weight of the batteries, and (b) incorporating high energy density electrode materials. By incorporating CNMs, the weight of the batteries was reduced by 5-10 times due to low mass loading of

Hardness enhancement and crosslinking mechanisms in polystyrene irradiated with high energy ion-beams

International Nuclear Information System (INIS)

Lee, E.H.; Rao, G.R.; Mansur, L.K.

1996-01-01

Surface hardness values several times larger than steel were produced using high energy ion beams at several hundred keV to MeV. High LET is important for crosslinking. Crosslinking is studied by analyzing hardness variations in response to irradiation parameter such as ion species, energy, and fluence. Effective crosslinking radii at hardness saturation are derived base on experimental data for 350 keV H + and 1 MeV Ar + irradiation of polystyrene. Saturation value for surface hardness is about 20 GPa

High-ion temperature experiments with negative-ion-based NBI in LHD

International Nuclear Information System (INIS)

Takeiri, Y.; Morita, S.; Tsumori, K.; Ikeda, K.; Oka, Y.; Osakabe, M.; Nagaoka, K.; Goto, M.; Miyazawa, J.; Masuzaki, S.; Ashikawa, N.; Yokoyama, M.; Narihara, K.; Yamada, I.; Kubo, S.; Shimozuma, T.; Inagaki, S.; Tanaka, K.; Peterson, B.J.; Ida, K.; Kaneko, O.; Komori, A.; Murakami, S.

2005-01-01

High-Z plasmas have been produced with Ar- and/or Ne-gas fuelling to increase the ion temperature in the LHD plasmas heated with the high-energy negative-ion-based NBI. Although the electron heating is dominant in the high-energy NBI heating, the direct ion heating power is much enhanced effectively in low-density plasmas due to both an increase in the beam absorption (ionisation) power and a reduction of the ion density in the high-Z plasmas. Intensive Ne- and/or Ar-glow discharge cleaning works well to suppress dilution of the high-Z plasmas with the wall-absorbed hydrogen. As a result, the ion temperature increases with an increase in the ion heating power normalized by the ion density, and reaches 10 keV. An increase in the ion temperature is also observed with an addition of the centrally focused ECRH to the low-density and high-Z NBI plasma, suggesting improvement of the ion transport. The results obtained in the high-Z plasma experiments with the high-energy NBI heating indicate that an increase in the direct ion heating power and improvement of the ion transport are essential to the ion temperature rise, and that a high-ion temperature would be obtained as well in hydrogen plasmas with low-energy positive-NBI heating which is planed in near future in LHD. (author)

Some general scaling rules in high energy heavy ion reactions

International Nuclear Information System (INIS)

Andersson, B.; Idh, J.; Otterlund, I.; Stenlund, E.

1988-09-01

We show, using the Fritiof model scenario that the wide variation in the number of participating nucleons tend to drown other dynamical variations in the measurables of high energy ion collisions. We propose a set if general scaling laws for inclusive distributions in which it is the mean multiplicity and the mean transverse energy from each source which are the measurables in the interactions. (authors)

Spectral measurements of few-electron uranium ions produced and trapped in a high-energy electron beam ion trap

International Nuclear Information System (INIS)

Beiersdorfer, P.

1994-01-01

Measurements of 2s l/2 -2p 3/2 electric dipole and 2p 1/2 -2p 3/2 magnetic dipole and electric quadrupole transitions in U 82+ through U 89+ have been made with a high-resolution crystal spectrometer that recorded the line radiation from stationary ions produced and trapped in a high-energy electron beam ion trap. From the measurements we infer -39.21 ± 0.23 eV for the QED contribution to the 2s 1/2 -2p 3/2 transition energy of lithiumlike U 89+ . A comparison between our measurements and various computations illustrates the need for continued improvements in theoretical approaches for calculating the atomic structure of ions with two or more electrons in the L shell

Corrosion behavior of low energy, high temperature nitrogen ion ...

Indian Academy of Sciences (India)

Corrosion behavior of low energy, high temperature nitrogen ion-implanted AISI 304 stainless steel. M GHORANNEVISS1, A SHOKOUHY1,∗, M M LARIJANI1,2,. S H HAJI HOSSEINI 1, M YARI1, A ANVARI4, M GHOLIPUR SHAHRAKI1,3,. A H SARI1 and M R HANTEHZADEH1. 1Plasma Physics Research Center, Science ...

Hydrogen microscopy and analysis of DNA repair using focused high energy ion beams

Energy Technology Data Exchange (ETDEWEB)

Dollinger, G. [Universitaet der Bundeswehr Muenchen, LRT 2, Werner Heisenberg Weg 39, D-85579 Neubiberg (Germany)]. E-mail: guenther.dollinger@unibw.de; Bergmaier, A. [Universitaet der Bundeswehr Muenchen, LRT 2, Werner Heisenberg Weg 39, D-85579 Neubiberg (Germany); Hauptner, A. [Physik Department E 12, Technische Universitaet Muenchen, D-85748 Garching (Germany); Dietzel, S. [Department Biologie II, Ludwigs-Maximilians-Universitaet Muenchen, Grosshaderner Str. 2, 82152 Planegg-Martinsried (Germany); Drexler, G.A. [Strahlenbiologisches Institut, LMU Muenchen, Schillerstr. 42, D-80336 Muenchen und Institut fuer Strahlenbiologie, GSF-Forschungszentrum, D-85764 Neuherberg (Germany); Greubel, C. [Physik Department E 12, Technische Universitaet Muenchen, D-85748 Garching (Germany); Hable, V. [Universitaet der Bundeswehr Muenchen, LRT 2, Werner Heisenberg Weg 39, D-85579 Neubiberg (Germany); Reichart, P. [School of Physics, University of Melbourne, Victoria 3010 (Australia); Kruecken, R. [Physik Department E 12, Technische Universitaet Muenchen, D-85748 Garching (Germany); Cremer, T. [Department Biologie II, Ludwigs-Maximilians-Universitaet Muenchen, Grosshaderner Str. 2, 82152 Planegg-Martinsried (Germany); Friedl, A.A. [Strahlenbiologisches Institut, LMU Muenchen, Schillerstr. 42, D-80336 Muenchen und Institut fuer Strahlenbiologie, GSF-Forschungszentrum, D-85764 Neuherberg (Germany)

2006-08-15

The ion microprobe SNAKE (Supraleitendes Nanoskop fuer Angewandte Kernphysikalische Experimente) at the Munich 14 MV tandem accelerator achieves beam focussing by a superconducting quadrupole doublet and can make use of a broad range of ions and ion energies, i.e. 4-28 MeV protons or up to 250 MeV gold ions. Due to these ion beams, SNAKE is particularly attractive for ion beam analyses in various fields. Here we describe two main applications of SNAKE. One is the unique possibility to perform three-dimensional hydrogen microscopy by elastic proton-proton scattering utilizing high energy proton beams. The high proton energies allow the analysis of samples with a thickness in the 100 {mu}m range with micrometer resolution and a sensitivity better than 1 ppm. In a second application, SNAKE is used to analyse protein dynamics in cells by irradiating live cells with single focussed ions. Fluorescence from immunostained protein 53BP1 is used as biological track detector after irradiation of HeLa cells. It is used to examine the irradiated region in comparison with the targeted region. Observed patterns of fluorescence foci agree reasonably well with irradiation patterns, indicating an overall targeting accuracy of about 2 {mu}m while the beam spot size is less than 0.5 {mu}m in diameter. This performance shows successful adaptation of SNAKE for biological experiments where cells are targeted on a sub-cellular level by energetic ions.

Microscopic descriptions of high-energy heavy-ion collisions

International Nuclear Information System (INIS)

Bodmer, A.R.

1977-01-01

The essentials of the equation-of-motion (EOM) approach are given and some of its significant and interesting results are described. A framework for the theoretical description of high-energy heavy-ion (HE-HI) collisions is presented; specifically included are a critical assessment of various approaches--EOM calculations, Boltzmann equations/cascade calculations, and hydrodynamics--their relationships and their respective domains of applicability, if any, to HE-HI collisions. 11 figures, 3 tables

Lamb shift measurement in hydrogenlike phosphorus

International Nuclear Information System (INIS)

Mueller, D.; Gassen, J.; Kremer, L.

1988-01-01

In hydrogenlike phosphorus ions the 2S 1/2 -2P 1/2 energy splitting (Lamb shift) has been found to be E exp (LS)=0.08343(29) eV using laser spectroscopy. This result is to be compared with the most recent theoretical value E th (LS)=0.08376(4) eV by Mohr and Johnson and Soff

Searching for squeezed particle-antiparticle correlations in high-energy heavy-ion collisions

International Nuclear Information System (INIS)

Padula, Sandra S.; Socolowski, O. Jr.

2010-01-01

Squeezed correlations of particle-antiparticle pairs were predicted to exist if the hadron masses were modified in the hot and dense medium formed in high-energy heavy-ion collisions. Although well-established theoretically, they have not yet been observed experimentally. We suggest here a clear method to search for such a signal by analyzing the squeezed correlation functions in terms of measurable quantities. We illustrate this suggestion for simulated φφ pairs at the Relativistic Heavy Ion Collider (RHIC) energies.

Unique aqueous Li-ion/sulfur chemistry with high energy density and reversibility.

Science.gov (United States)

Yang, Chongyin; Suo, Liumin; Borodin, Oleg; Wang, Fei; Sun, Wei; Gao, Tao; Fan, Xiulin; Hou, Singyuk; Ma, Zhaohui; Amine, Khalil; Xu, Kang; Wang, Chunsheng

2017-06-13

Leveraging the most recent success in expanding the electrochemical stability window of aqueous electrolytes, in this work we create a unique Li-ion/sulfur chemistry of both high energy density and safety. We show that in the superconcentrated aqueous electrolyte, lithiation of sulfur experiences phase change from a high-order polysulfide to low-order polysulfides through solid-liquid two-phase reaction pathway, where the liquid polysulfide phase in the sulfide electrode is thermodynamically phase-separated from the superconcentrated aqueous electrolyte. The sulfur with solid-liquid two-phase exhibits a reversible capacity of 1,327 mAh/(g of S), along with fast reaction kinetics and negligible polysulfide dissolution. By coupling a sulfur anode with different Li-ion cathode materials, the aqueous Li-ion/sulfur full cell delivers record-high energy densities up to 200 Wh/(kg of total electrode mass) for >1,000 cycles at ∼100% coulombic efficiency. These performances already approach that of commercial lithium-ion batteries (LIBs) using a nonaqueous electrolyte, along with intrinsic safety not possessed by the latter. The excellent performance of this aqueous battery chemistry significantly promotes the practical possibility of aqueous LIBs in large-format applications.

DIAGNOSTICS FOR ION BEAM DRIVEN HIGH ENERGY DENSITY PHYSICS EXPERIMENTS

International Nuclear Information System (INIS)

Bieniosek, F.M.; Henestroza, E.; Lidia, S.; Ni, P.A.

2010-01-01

Intense beams of heavy ions are capable of heating volumetric samples of matter to high energy density. Experiments are performed on the resulting warm dense matter (WDM) at the NDCX-I ion beam accelerator. The 0.3 MeV, 30-mA K + beam from NDCX-I heats foil targets by combined longitudinal and transverse neutralized drift compression of the ion beam. Both the compressed and uncompressed parts of the NDCX-I beam heat targets. The exotic state of matter (WDM) in these experiments requires specialized diagnostic techniques. We have developed a target chamber and fielded target diagnostics including a fast multi-channel optical pyrometer, optical streak camera, laser Doppler-shift interferometer (VISAR), beam transmission diagnostics, and high-speed gated cameras. We also present plans and opportunities for diagnostic development and a new target chamber for NDCX-II.

Jet and Leading Hadron Production in High-energy Heavy-ion Collisions

International Nuclear Information System (INIS)

Wang, Xin-Nian

2005-01-01

Jet tomography has become a powerful tool for the study of properties of dense matter in high-energy heavy-ion collisions. I will discuss recent progresses in the phenomenological study of jet quenching, including momentum, colliding energy and nuclear size dependence of single hadron suppression, modification of dihadron correlations and the soft hadron distribution associated with a quenched jet

Nanomaterials Enabled High Energy and Power Density Li-ion Batteries, Phase I

Data.gov (United States)

National Aeronautics and Space Administration — There is a need for high energy (~ 200 Wh/kg) and high power (> 500 W/kg) density rechargeable Li-ion batteries that are safe and reliable for several space and...

High Energy Density Li-ion Cells for EV’s Based on Novel, High Voltage Cathode Material Systems

Energy Technology Data Exchange (ETDEWEB)

Kepler, Keith [Farasis Energy Inc; Slater, Michael [Farasis Energy Inc

2018-03-14

This Li-ion cell technology development project had three objectives: to develop advanced electrode materials and cell components to enable stable high-voltage operation; to design and demonstrate a Li-ion cell using these materials that meets the PHEV40 performance targets; and to design and demonstrate a Li-ion cell using these materials that meets the EV performance targets. The major challenge to creating stable high energy cells with long cycle life is system integration. Although materials that can give high energy cells are known, stabilizing them towards long-term cycling in the presence of other novel cell components is a major challenge. The major technical barriers addressed by this work include low cathode specific energy, poor electrolyte stability during high voltage operation, and insufficient capacity retention during deep discharge for Si-containing anodes. Through the course of this project, Farasis was able to improve capacity retention of NCM materials for 4.4+ V operation, through both surface treatment and bulk-doping approaches. Other material advances include increased rate capability and of HE-NCM materials through novel synthesis approach, doubling the relative capacity at 1C over materials synthesized using standard methods. Silicon active materials proved challenging throughout the project and ultimately were the limiting factor in the energy density vs. cycle life trade off. By avoiding silicon anodes for the lower energy PHEV design, we manufactured cells with intermediate energy density and long cycle life under high voltage operation for PHEV applications. Cells with high energy density for EV applications were manufactured targeting a 300 Wh/kg design and were able to achieve > 200 cycles.

Feasibility of Cathode Surface Coating Technology for High-Energy Lithium-ion and Beyond-Lithium-ion Batteries.

Science.gov (United States)

Kalluri, Sujith; Yoon, Moonsu; Jo, Minki; Liu, Hua Kun; Dou, Shi Xue; Cho, Jaephil; Guo, Zaiping

2017-12-01

Cathode material degradation during cycling is one of the key obstacles to upgrading lithium-ion and beyond-lithium-ion batteries for high-energy and varied-temperature applications. Herein, we highlight recent progress in material surface-coating as the foremost solution to resist the surface phase-transitions and cracking in cathode particles in mono-valent (Li, Na, K) and multi-valent (Mg, Ca, Al) ion batteries under high-voltage and varied-temperature conditions. Importantly, we shed light on the future of materials surface-coating technology with possible research directions. In this regard, we provide our viewpoint on a novel hybrid surface-coating strategy, which has been successfully evaluated in LiCoO 2 -based-Li-ion cells under adverse conditions with industrial specifications for customer-demanding applications. The proposed coating strategy includes a first surface-coating of the as-prepared cathode powders (by sol-gel) and then an ultra-thin ceramic-oxide coating on their electrodes (by atomic-layer deposition). What makes it appealing for industry applications is that such a coating strategy can effectively maintain the integrity of materials under electro-mechanical stress, at the cathode particle and electrode- levels. Furthermore, it leads to improved energy-density and voltage retention at 4.55 V and 45 °C with highly loaded electrodes (≈24 mg.cm -2 ). Finally, the development of this coating technology for beyond-lithium-ion batteries could be a major research challenge, but one that is viable. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Advanced Electrode Materials for High Energy Next Generation Li ion Batteries

Science.gov (United States)

Hayner, Cary Michael

Lithium ion batteries are becoming an increasingly ubiquitous part of modern society. Since their commercial introduction by Sony in 1991, lithium-ion batteries have grown to be the most popular form of electrical energy storage for portable applications. Today, lithium-ion batteries power everything from cellphones and electric vehicles to e-cigarettes, satellites, and electric aircraft. Despite the commercialization of lithium-ion batteries over twenty years ago, it remains the most active field of energy storage research for its potential improvement over current technology. In order to capitalize on these opportunities, new materials with higher energy density and storage capacities must be developed. Unfortunately, most next-generation materials suffer from rapid capacity degradation or severe loss of capacity when rapidly discharged. In this dissertation, the development of novel anode and cathode materials for advanced high-energy and high-power lithium-ion batteries is reported. In particular, the application of graphene-based materials to stabilize active material is emphasized. Graphene, a unique two-dimensional material composed of atomically thin carbon sheets, has shown potential to address unsatisfactory rate capability, limited cycling performance and abrupt failure of these next-generation materials. This dissertation covers four major subjects: development of silicon-graphene composites, impact of carbon vacancies on graphene high-rate performance, iron fluoride-graphene composites, and ternary iron-manganese fluoride synthesis. Silicon is considered the most likely material to replace graphite as the anode active material for lithium-ion batteries due to its ability to alloy with large amounts of lithium, leading to significantly higher specific capacities than the graphite standard. However, Si also expands in size over 300% upon lithiation, leading to particle fracture and isolation from conductive support, resulting in cell failure within a few

High energy (MeV) ion-irradiated π-conjugated polyaniline: Transition from insulating state to carbonized conducting state

International Nuclear Information System (INIS)

Park, S.K.; Lee, S.Y.; Lee, C.S.; Kim, H.M.; Joo, J.; Beag, Y.W.; Koh, S.K.

2004-01-01

High energy (MeV) C 2+ , F 2+ , and Cl 2+ ions were irradiated onto π-conjugated polyaniline emeraldine base (PAN-EB) samples. The energy of an ion beam was controlled to a range of 3-4.5 MeV, with the ion dosage varying from 1x10 12 to 1x10 16 ions/cm 2 . The highest dc conductivity (σ dc ) at room temperature was measured to be ∼60 S/cm for 4.5 MeV Cl 2+ ion-irradiated PAN-EB samples with a dose of 1x10 16 ions/cm 2 . We observed the transition of high energy ion-irradiated PAN-EB samples from insulating state to conducting state as a function of ion dosage based on σ dc and its temperature dependence. The characteristic peaks of the Raman spectrum of the PAN-EB samples were reduced, while the D-peak (disordered peak) and the G peak (graphitic peak) appeared as the ion dose increased. From the analysis of the D and G peaks of the Raman spectra of the systems compared to multiwalled carbon nanotubes, ion-irradiated graphites, and annealed carbon films, the number of the clusters of hexagon rings with conducting sp 2 -bonded carbons increased with ion dosage. We also observed the increase in the size of the nanocrystalline graphitic domain of the systems with increasing ion dosage. The intensity of normalized electron paramagnelic resonance signal also increased in correlation with ion dose. The results of this study demonstrate that π-conjugated pristine PAN-EB systems changed from insulating state to carbonized conducting state through high energy ion irradiation with high ion dosage

Binding energies of cluster ions

International Nuclear Information System (INIS)

Parajuli, R.; Matt, S.; Scheier, P.; Echt, O.; Stamatovic, A.; Maerk, T.D.

2002-01-01

The binding energy of charged clusters may be measured by analyzing the kinetic energy released in the metastable decay of mass selected parent ions. Using finite heat bath theory to determine the binding energies of argon, neon, krypton, oxygen and nitrogen from their respective average kinetic energy released were carried out. A high-resolution double focussing two-sector mass spectrometer of reversed Nier-Johnson type geometry was used. MIKE ( mass-analysed ion kinetic energy) were measured to investigate decay reactions of mass-selected ions. For the inert gases neon (Ne n + ), argon (Ar n + ) and krypton (Kr n + ), it is found that the binding energies initially decrease with increasing size n and then level off at a value above the enthalpy of vaporization of the condensed phase. Oxygen cluster ions shown a characteristic dependence on cluster size (U-shape) indicating a change in the metastable fragmentation mechanism when going from the dimer to the decamer ion. (nevyjel)

Measurement of residual radioactivity in cooper exposed to high energy heavy ion beam

Energy Technology Data Exchange (ETDEWEB)

Kim, Eunjoo; Nakamura, Takashi [Tohoku Univ., Sendai (Japan). Cyclotron and Radioisotope Center; Uwamino, Yoshitomo; Ito, Sachiko; Fukumura, Akifumi

1999-03-01

The residual radioactivities produced by high energy heavy ions have been measured using the heavy ion beams of the Heavy Ion Medical Accelerator (HIMAC) at National Institute of Radiological Sciences. The spatial distribution of residual radioactivities in 3.5 cm, 5.5 cm and 10 cm thick copper targets of 10 cm x 10 cm size bombarded by 290 MeV/u, 400 MeV/u-{sup 12}C ion beams and 400 MeV/u-{sup 20}Ne ion beam, respectively, were obtained by measuring the gamma-ray activities of 0.5 mm thick copper foil inserted in the target with a high purity Ge detector after about 1 hour to 6 hours irradiation. (author)

Supported black phosphorus nanosheets as hydrogen-evolving photocatalyst achieving 5.4% energy conversion efficiency at 353 K.

Science.gov (United States)

Tian, Bin; Tian, Bining; Smith, Bethany; Scott, M C; Hua, Ruinian; Lei, Qin; Tian, Yue

2018-04-11

Solar-driven water splitting using powdered catalysts is considered as the most economical means for hydrogen generation. However, four-electron-driven oxidation half-reaction showing slow kinetics, accompanying with insufficient light absorption and rapid carrier combination in photocatalysts leads to low solar-to-hydrogen energy conversion efficiency. Here, we report amorphous cobalt phosphide (Co-P)-supported black phosphorus nanosheets employed as photocatalysts can simultaneously address these issues. The nanosheets exhibit robust hydrogen evolution from pure water (pH = 6.8) without bias and hole scavengers, achieving an apparent quantum efficiency of 42.55% at 430 nm and energy conversion efficiency of over 5.4% at 353 K. This photocatalytic activity is attributed to extremely efficient utilization of solar energy (~75% of solar energy) by black phosphorus nanosheets and high-carrier separation efficiency by amorphous Co-P. The hybrid material design realizes efficient solar-to-chemical energy conversion in suspension, demonstrating the potential of black phosphorus-based materials as catalysts for solar hydrogen production.

High current density ion beam obtained by a transition to a highly focused state in extremely low-energy region

Energy Technology Data Exchange (ETDEWEB)

Hirano, Y., E-mail: y.hirano@aist.go.jp, E-mail: hirano.yoichi@phys.cst.nihon-u.ac.jp [Innovative Plasma Processing Group, National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki 305-8568 (Japan); College of Science and Technologies, Nihon University, Chiyodaku, Tokyo 101-0897 (Japan); Kiyama, S.; Koguchi, H. [Innovative Plasma Processing Group, National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki 305-8568 (Japan); Fujiwara, Y.; Sakakita, H. [Innovative Plasma Processing Group, National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki 305-8568 (Japan); Department of Engineering Mechanics and Energy, University of Tsukuba, Ibaraki 305-8577 (Japan)

2015-11-15

A high current density (≈3 mA/cm{sup 2}) hydrogen ion beam source operating in an extremely low-energy region (E{sub ib} ≈ 150–200 eV) has been realized by using a transition to a highly focused state, where the beam is extracted from the ion source chamber through three concave electrodes with nominal focal lengths of ≈350 mm. The transition occurs when the beam energy exceeds a threshold value between 145 and 170 eV. Low-level hysteresis is observed in the transition when E{sub ib} is being reduced. The radial profiles of the ion beam current density and the low temperature ion current density can be obtained separately using a Faraday cup with a grid in front. The measured profiles confirm that more than a half of the extracted beam ions reaches the target plate with a good focusing profile with a full width at half maximum of ≈3 cm. Estimation of the particle balances in beam ions, the slow ions, and the electrons indicates the possibility that the secondary electron emission from the target plate and electron impact ionization of hydrogen may play roles as particle sources in this extremely low-energy beam after the compensation of beam ion space charge.

Coherent production of high-energy photons and π mesons in heavy ion reactions

International Nuclear Information System (INIS)

Batkin, I.S.; Kopytin, I.V.

1986-01-01

A microscopic model of high-energy photon and pion production processes in collision of multicharged ions with kinetic energy of relative motion from 40 to 100 MeV per nucleon was constructed not using fitting parameters

Fabrication and Characterization of Li-ion Electrodes for High-Power Energy Storage Devices

OpenAIRE

Lai, Chun-Han

2017-01-01

Renewable energy technologies have been a rapidly emerging option to meet future energy demand. However, their systems require stable, high-power storage devices to overcome fluctuating energy outputs for consistent distribution. Since traditional Li-ion batteries (LIB) are not considered to be capable of fast charging and discharging, we have to develop devices with new chemistry for high-power operation. This dissertation focuses on the development of supercapacitors and high-rate batteries...

Tailored ion energy distributions on plasma electrodes

International Nuclear Information System (INIS)

Economou, Demetre J.

2013-01-01

As microelectronic device features continue to shrink approaching atomic dimensions, control of the ion energy distribution on the substrate during plasma etching and deposition becomes increasingly critical. The ion energy should be high enough to drive ion-assisted etching, but not too high to cause substrate damage or loss of selectivity. In many cases, a nearly monoenergetic ion energy distribution (IED) is desired to achieve highly selective etching. In this work, the author briefly reviews: (1) the fundamentals of development of the ion energy distribution in the sheath and (2) methods to control the IED on plasma electrodes. Such methods include the application of “tailored” voltage waveforms on an electrode in continuous wave plasmas, or the application of synchronous bias on a “boundary electrode” during a specified time window in the afterglow of pulsed plasmas

Chemical modification of polypropylene induced by high energy carbon ions

Energy Technology Data Exchange (ETDEWEB)

Saha, A.; Chakraborty, V.; Chintalapudi, S.N. E-mail: snc@gamma.iuc.res.in

2000-06-01

Polypropylene was irradiated with {sup 12}C{sup +} ions of 3.6 and 5.4 MeV energy using 3 MV Pelletron. The spectral changes owing to ion bombardment were investigated by UV-VIS and Fourier-transform infrared (FTIR) spectroscopy. A gradual increase in absorbance was observed around visible and near visible region with increase in fluence of bombarding ions. The difference absorption spectra show formation of chromophoric groups with wavelength maximum near 380 nm at lower fluence, but at high fluence a shift in peak is observed. The chromophoric groups are likely to be the extended conjugated polyene system and the red shift in peak position at high fluence may be attributed to the greater degree of conjugation. The formation of unsaturated linkage is confirmed by the FTIR spectra with observed stretching band around 1650 cm{sup -1} and its intensity was found to increase with increase in ion fluence studied. The gases (in the range 2-80 amu) which were evolved due to interaction of polypropylene with {sup 12}C{sup +} ions were measured with Residual Gas Analyzer (RGA). A large number of gaseous components were detected. This shows that polymer chains break into some smaller fragments which concomitantly leads to extended conjugation.

Effect of phosphorus on hot ductility of high purity iron

International Nuclear Information System (INIS)

Abiko, K.; Liu, C.M.; Ichikawa, M..; Suenaga, H.; Tanino, M.

1995-01-01

Tensile tests on high purity Fe-P alloys with 0, 0.05 and 0.1 mass%P were carried out at temperatures between 300 K and 1073 K to clarify the intrinsic effect of phosphorus on the mechanical properties of iron at elevated temperatures. Microstructures of as-quenched, interrupted and ruptured specimens were observed. Experimental results show that the addition of phosphorus causes a remarkable increase in proof stress of high purity iron at 300 K, but the increase in proof stress by phosphorus decreases with increasing test temperature. The strengthening effect of phosphorus reduces to zero at 1073 K. High purity iron and Fe-P alloys rupture at almost 100% reduction in area at the whole test temperatures. However, Fe-P alloys show much larger elongation at test temperatures above 773 K than high purity iron. The increased elongation of high purity iron by addition of phosphorus was shown to be related to the effect of phosphorus on dynamic recovery and recrystallization of iron as its intrinsic effect. (orig.)

Characterisation Of The Beam Plasma In High Current, Low Energy Ion Beams For Implanters

International Nuclear Information System (INIS)

Fiala, J.; Armour, D. G.; Berg, J. A. van der; Holmes, A. J. T.; Goldberg, R. D.; Collart, E. H. J.

2006-01-01

The effective transport of high current, positive ion beams at low energies in ion implanters requires the a high level of space charge compensation. The self-induced or forced introduction of electrons is known to result in the creation of a so-called beam plasma through which the beam propagates. Despite the ability of beams at energies above about 3-5 keV to create their own neutralising plasmas and the development of highly effective, plasma based neutralising systems for low energy beams, very little is known about the nature of beam plasmas and how their characteristics and capabilities depend on beam current, beam energy and beamline pressure. These issues have been addressed in a detailed scanning Langmuir probe study of the plasmas created in beams passing through the post-analysis section of a commercial, high current ion implanter. Combined with Faraday cup measurements of the rate of loss of beam current in the same region due to charge exchange and scattering collisions, the probe data have provided a valuable insight into the nature of the slow ion and electron production and loss processes. Two distinct electron energy distribution functions are observed with electron temperatures ≥ 25 V and around 1 eV. The fast electrons observed must be produced in their energetic state. By studying the properties of the beam plasma as a function of the beam and beamline parameters, information on the ways in which the plasma and the beam interact to reduce beam blow-up and retain a stable plasma has been obtained

High yield antibiotic producing mutants of Streptomyces erythreus induced by low energy ion implantation

Science.gov (United States)

Yu, Chen; Zhixin, Lin; Zuyao, Zou; Feng, Zhang; Duo, Liu; Xianghuai, Liu; Jianzhong, Tang; Weimin, Zhu; Bo, Huang

1998-05-01

Conidia of Streptomyces erythreus, an industrial microbe, were implanted by nitrogen ions with energy of 40-60 keV and fluence from 1 × 10 11 to 5 × 10 14 ions/cm 2. The logarithm value of survival fraction had good linear relationship with the logarithm value of fluence. Some mutants with a high yield of erythromycin were induced by ion implantation. The yield increment was correlated with the implantation fluence. Compared with the mutation results induced by ultraviolet rays, mutation effects of ion implantation were obvious having higher increasing erythromycin potency and wider mutation spectrum. The spores of Bacillus subtilis were implanted by arsenic ions with energy of 100 keV. The distribution of implanted ions was measured by Rutherford Backscattering Spectrometry (RBS) and calculated in theory. The mechanism of mutation induced by ion implantation was discussed.

Energy dissipation on ion-accelerator grids during high-voltage breakdown

International Nuclear Information System (INIS)

Menon, M.M.; Ponte, N.S.

1981-01-01

The effects of stored energy in the system capacitance across the accelerator grids during high voltage vacuum breakdown are examined. Measurements were made of the current flow and the energy deposition on the grids during breakdown. It is shown that only a portion (less than or equal to 40 J) of the total stored energy (congruent to 100 J) is actually dissipated on the grids. Most of the energy is released during the formation phase of the vacuum arc and is deposited primarily on the most positive grid. Certain abnormal situations led to energy depositions of about 200 J on the grid, but the ion accelerator endured them without exhibiting any deterioration in performance

Scintillation screen materials for beam profile measurements of high energy ion beams

Energy Technology Data Exchange (ETDEWEB)

Krishnakumar, Renuka

2016-06-22

For the application as a transverse ion beam diagnostics device, various scintillation screen materials were analysed. The properties of the materials such as light output, image reproduction and radiation stability were investigated with the ion beams extracted from heavy ion synchrotron SIS-18. The ion species (C, Ne, Ar, Ta and U) were chosen to cover the large range of elements in the periodic table. The ions were accelerated to the kinetic energies of 200 MeV/u and 300 MeV/u extracted with 300 ms pulse duration and applied to the screens. The particle intensity of the ion beam was varied from 10{sup 4} to 10{sup 9} particles per pulse. The screens were irradiated with typically 40 beam pulses and the scintillation light was captured using a CCD camera followed by characterization of the beam spot. The radiation hardness of the screens was estimated with high intensity Uranium ion irradiation. In the study, a linear light output for 5 orders of magnitude of particle intensities was observed from sensitive scintillators and ceramic screens such as Al{sub 2}O{sub 3}:Cr and Al{sub 2}O{sub 3}. The highest light output was recorded by CsI:Tl and the lowest one by Herasil. At higher beam intensity saturation of light output was noticed from Y and Mg doped ZrO{sub 2} screens. The light output from the screen depends not only on the particle intensity but also on the ion species used for irradiation. The light yield (i.e. the light intensity normalised to the energy deposition in the material by the ion) is calculated from the experimental data for each ion beam setting. It is shown that the light yield for light ions is about a factor 2 larger than the one of heavy ions. The image widths recorded exhibit a dependence on the screens material and differences up to 50 % were registered. On radiation stability analysis with high particle intensity of Uranium ions of about 6 x 10{sup 8} ppp, a stable performance in light output and image reproduction was documented from Al

Laser - driven high - energy ions and their application to inertial confinement fusion

International Nuclear Information System (INIS)

Borghesi, M.

2007-01-01

The acceleration of high-energy ion beams (up to several tens of MeV per nucleon) following the interaction of short and intense laser pulses with solid targets has been one of the most important results of recent laser-plasma research [1]. The acceleration is driven by relativistic electrons, which acquire energy directly from the laser pulse and set up extremely large (∼TV/m) space charge fields at the target interfaces. The properties of laser-driven ion beams (high brightness and laminarity, high-energy cut-off, ultrashort burst duration) distinguish them from lower energy ions accelerated in earlier experiments at moderate laser intensities, and compare favourably with those of 'conventional' accelerator beams. In view of these properties, laser-driven ion beams can be employed in a number of innovative applications in the scientific, technological and medical areas. We will discuss in particular aspects of interest to their application in an Inertial Confinement Fusion context. Laser-driven protons are indeed being considered as a possible trigger for Fast Ignition of a precompressed fuel.[2] Recent results relating to the optimization of beam energy and focusing will be presented. These include the use of laser-driven impulsive fields for proton beam collimation and focusing [3], and the investigation of acceleration in presence of finite-scale plasma gradient. Proposed target developments enabling proton production at high repetition rate will also be discussed. Another important area of application of proton beams is diagnostic use in a particle probing arrangement for detection of density non-homogeneities [4] and electric/magnetic fields [5]. We will discuss the use of laser-driven proton beams for the diagnosis of magnetic and electric fields in planar and hohlraum targets and for the detection of fields associated to relativistic electron propagation through dense matter, an issue of high relevance for electron driven Fast Ignition. [1] M

HIGH ENERGY DENSITY PHYSICS EXPERIMENTS WITH INTENSE HEAVY ION BEAMS

International Nuclear Information System (INIS)

Bieniosek, F.M.; Henestroza, E.; Leitner, M.; Logan, B.G.; More, R.M.; Roy, P.K.; Ni, P.; Seidl, P.A.; Waldron, W.L.; Barnard, J.J.

2008-01-01

The US heavy ion fusion science program has developed techniques for heating ion-beam-driven warm dense matter (WDM) targets. The WDM conditions are to be achieved by combined longitudinal and transverse space-charge neutralized drift compression of the ion beam to provide a hot spot on the target with a beam spot size of about 1 mm, and pulse length about 1-2 ns. As a technique for heating volumetric samples of matter to high energy density, intense beams of heavy ions are capable of delivering precise and uniform beam energy deposition dE/dx, in a relatively large sample size, and the ability to heat any solid-phase target material. Initial experiments use a 0.3 MeV K+ beam (below the Bragg peak) from the NDCX-I accelerator. Future plans include target experiments using the NDCX-II accelerator, which is designed to heat targets at the Bragg peak using a 3-6 MeV lithium ion beam. The range of the beams in solid matter targets is about 1 micron, which can be lengthened by using porous targets at reduced density. We have completed the fabrication of a new experimental target chamber facility for WDM experiments, and implemented initial target diagnostics to be used for the first target experiments in NDCX-1. The target chamber has been installed on the NDCX-I beamline. The target diagnostics include a fast multi-channel optical pyrometer, optical streak camera, VISAR, and high-speed gated cameras. Initial WDM experiments will heat targets by compressed NDCX-I beams and will explore measurement of temperature and other target parameters. Experiments are planned in areas such as dense electronegative targets, porous target homogenization and two-phase equation of state

Pulse-height response of silicon surface-barrier detectors to high-energy heavy ions

International Nuclear Information System (INIS)

Smith, G.D.

1973-01-01

The pulse-height defect (PHD) of high-energy heavy ions in silicon surface-barrier detectors can be divided into three components: (1) energy loss in the gold-surface layer, (2) a nuclear-stopping defect, and (3) a defect due to recombination of electron-hole pairs in the plasma created by the heavy ion. The plasma recombination portion of the PHD was the subject of this study using the variation of the PHD with (1) the angle of incidence of incoming heavy ions, and (2) changes in the detector bias. The Tandem Van de Graaff accelerator at Argonne National Laboratory was used to produce scattered beam ions ( 32 S, 35 Cl) and heavy target recoils (Ni, Cu, 98 Mo, Ag, Au) at sufficient energies to produce a significant recombination defect. The results confirm the existence of a recombination zone at the front surface of these detectors and the significance of plasma recombination as a portion of the pulse-height defect. (Diss. Abstr. Int., B)

Calibration of BAS-TR image plate response to high energy (3-300 MeV) carbon ions

Science.gov (United States)

Doria, D.; Kar, S.; Ahmed, H.; Alejo, A.; Fernandez, J.; Cerchez, M.; Gray, R. J.; Hanton, F.; MacLellan, D. A.; McKenna, P.; Najmudin, Z.; Neely, D.; Romagnani, L.; Ruiz, J. A.; Sarri, G.; Scullion, C.; Streeter, M.; Swantusch, M.; Willi, O.; Zepf, M.; Borghesi, M.

2015-12-01

The paper presents the calibration of Fuji BAS-TR image plate (IP) response to high energy carbon ions of different charge states by employing an intense laser-driven ion source, which allowed access to carbon energies up to 270 MeV. The calibration method consists of employing a Thomson parabola spectrometer to separate and spectrally resolve different ion species, and a slotted CR-39 solid state detector overlayed onto an image plate for an absolute calibration of the IP signal. An empirical response function was obtained which can be reasonably extrapolated to higher ion energies. The experimental data also show that the IP response is independent of ion charge states.

High Energy Density Solid State Li-ion Battery with Enhanced Safety, Phase I

Data.gov (United States)

National Aeronautics and Space Administration — We propose to develop an all solid state Li-ion battery which is capable of delivering high energy density, combined with high safety over a wide operating...

DYNAMICS OF HIGH ENERGY IONS AT A STRUCTURED COLLISIONLESS SHOCK FRONT

Energy Technology Data Exchange (ETDEWEB)

Gedalin, M. [Department of Physics, Ben-Gurion University of the Negev, Beer-Sheva (Israel); Dröge, W.; Kartavykh, Y. Y., E-mail: gedalin@bgu.ac.il [Institute for Theoretical Physics and Astrophysics, University of Würzburg, Würzburg (Germany)

2016-07-10

Ions undergoing first-order Fermi acceleration at a shock are scattered in the upstream and downstream regions by magnetic inhomogeneities. For high energy ions this scattering is efficient at spatial scales substantially larger than the gyroradius of the ions. The transition from one diffusive region to the other occurs via crossing the shock, and the ion dynamics during this crossing is mainly affected by the global magnetic field change between the upstream and downstream region. We study the effects of the fine structure of the shock front, such as the foot-ramp-overshoot profile and the phase-standing upstream and downstream magnetic oscillations. We also consider time dependent features, including reformation and large amplitude coherent waves. We show that the influence of the spatial and temporal structure of the shock front on the dependence of the transition and reflection on the pitch angle of the ions is already weak at ion speeds five times the speed of the upstream flow.

Measurement of energy deposition near high energy, heavy ion tracks. Progress report, December 1982-April 1985

Energy Technology Data Exchange (ETDEWEB)

Metting, N.F.; Braby, L.A.; Rossi, H.H.; Kliauga, P.J.; Howard, J.; Schimmerling, W.; Wong, M.; Rapkin, M.

1986-08-01

The microscopic spatial distribution of energy deposition in irradiated tissue plays a significant role in the final biological effect produced. Therefore, it is important to have accurate microdosimetric spectra of radiation fields used for radiobiology and radiotherapy. The experiments desribed here were designed to measure the distributions of energy deposition around high energy heavy ion tracks generated at Lawrence Berkeley Laboratory's Bevalac Biomedical Facility. A small proportional counter mounted in a large (0.6 by 2.5 m) vacuum chamber was used to measure energy deposition distributions as a function of the distance between detector and primary ion track. The microdosimetric distributions for a homogeneous radiation field were then calculated by integrating over radial distance. This thesis discusses the rationale of the experimental design and the analysis of measurements on 600 MeV/amu iron tracks. 53 refs., 19 figs.

Measurement of energy deposition near high energy, heavy ion tracks. Progress report, December 1982-April 1985

International Nuclear Information System (INIS)

Metting, N.F.; Braby, L.A.; Rossi, H.H.; Kliauga, P.J.; Howard, J.; Schimmerling, W.; Wong, M.; Rapkin, M.

1986-08-01

The microscopic spatial distribution of energy deposition in irradiated tissue plays a significant role in the final biological effect produced. Therefore, it is important to have accurate microdosimetric spectra of radiation fields used for radiobiology and radiotherapy. The experiments desribed here were designed to measure the distributions of energy deposition around high energy heavy ion tracks generated at Lawrence Berkeley Laboratory's Bevalac Biomedical Facility. A small proportional counter mounted in a large (0.6 by 2.5 m) vacuum chamber was used to measure energy deposition distributions as a function of the distance between detector and primary ion track. The microdosimetric distributions for a homogeneous radiation field were then calculated by integrating over radial distance. This thesis discusses the rationale of the experimental design and the analysis of measurements on 600 MeV/amu iron tracks. 53 refs., 19 figs

High-energy xenon ion irradiation effects on the electrical properties of yttrium iron garnet

International Nuclear Information System (INIS)

Costantini, J.M.; Flament, J.L.; Sinopoli, L.; Trochon, J.; Uzureau, J.L.; Groult, D.; Studer, F.; Toulemonde, M.

1989-01-01

Thin monocristalline samples of yttrium iron garnet Y 3 Fe 5 O 12 (YIG) were irradiated at room temperature with 27 MeV/A 132 Xe ions at varying fluences up to 3.5 x 10 12 ions cm -2 . Sample thickness (100 μm) was smaller than the mean projected range of ions (170 μm) so that we were able to study the effects of irradiation damage solely. At such a high ion energy the nuclear energy loss is negligible and damage is mainly due to electronic excitation energy loss. YIG d.c conductivity is found to rise by a factor 40 for the highest dose while the permittivity increases only slightly after irradiation (40% max.). The dielectric losses are also enhanced as the ion fluence increases especially at lower frequencies (by a factor 6 at 10 KHz). No dielectric relaxation peak is observed in the frequency range explored here (10 KHz - 10 MHz)

High-energy high-luminosity electron-ion collider eRHIC

International Nuclear Information System (INIS)

Litvinenko, V.N.; Ben-Zvi, I.; Hammons, L.; Hao, Y.; Webb, S.

2011-01-01

In this paper, we describe a future electron-ion collider (EIC), based on the existing Relativistic Heavy Ion Collider (RHIC) hadron facility, with two intersecting superconducting rings, each 3.8 km in circumference. The replacement cost of the RHIC facility is about two billion US dollars, and the eRHIC will fully take advantage and utilize this investment. We plan adding a polarized 5-30 GeV electron beam to collide with variety of species in the existing RHIC accelerator complex, from polarized protons with a top energy of 325 GeV, to heavy fully-striped ions with energies up to 130 GeV/u. Brookhaven's innovative design, is based on one of the RHIC's hadron rings and a multi-pass energy-recovery linac (ERL). Using the ERL as the electron accelerator assures high luminosity in the 10 33 -10 34 cm -2 sec -1 range, and for the natural staging of eRHIC, with the ERL located inside the RHIC tunnel. The eRHIC will provide electron-hadron collisions in up to three interaction regions. We detail the eRHIC's performance in Section 2. Since first paper on eRHIC paper in 2000, its design underwent several iterations. Initially, the main eRHIC option (the so-called ring-ring, RR, design) was based on an electron ring, with the linac-ring (LR) option as a backup. In 2004, we published the detailed 'eRHIC 0th Order Design Report' including a cost-estimate for the RR design. After detailed studies, we found that an LR eRHIC has about a 10-fold higher luminosity than the RR. Since 2007, the LR, with its natural staging strategy and full transparency for polarized electrons, became the main choice for eRHIC. In 2009, we completed technical studies of the design and dynamics for MeRHIC with 3-pass 4 GeV ERL. We learned much from this evaluation, completed a bottom-up cost estimate for this $350M machine, but then shelved the design. In the same year, we turned again to considering the cost-effective, all-in-tunnel six-pass ERL for our design of the high-luminosity eRHIC. In it

Intercalation Pseudocapacitance in Ultrathin VOPO4 Nanosheets: Toward High-Rate Alkali-Ion-Based Electrochemical Energy Storage.

Science.gov (United States)

Zhu, Yue; Peng, Lele; Chen, Dahong; Yu, Guihua

2016-01-13

There is a growing need for energy storage devices in numerous applications where a large amount of energy needs to be either stored or delivered quickly. The present paper details the study of alkali-ion intercalation pseudocapacitance in ultrathin VOPO4 nanosheets, which hold promise in high-rate alkali-ion based electrochemical energy storage. Starting from bulk VOPO4·2H2O chunks, VOPO4 nanosheets were obtained through simple ultrasonication in 2-propanol. These nanosheets as the cathode exhibit a specific capacity of 154 and 136 mAh/g (close to theoretical value 166 mAh/g) for lithium and sodium storage devices at 0.1 C and 100 and ∼70 mAh/g at 5 C, demonstrating their high rate capability. Moreover, the capacity retention is maintained at 90% for lithium ion storage and 73% for sodium ion storage after 500 cycles, showing their reasonable stability. The demonstrated alkali-ion intercalation pseudocapacitance represents a promising direction for developing battery materials with promising high rate capability.

High-energy particle emission from galena and pyrite bombarded with Cs and O ions

International Nuclear Information System (INIS)

Karpuzov, D.S.; McIntyre, N.S.

2002-01-01

The ejection of energetic particles during steady-state ion surface bombardment has been investigated by means of a dynamic computer simulation as well as in a secondary ion mass spectrometry (SIMS)/low-energy ion scattering from surfaces (LEIS) experiment. The emphasis of this comparative study is on the mass dependence of high-energy tails in sputtering and backscattering for the bombardment of galena (PbS) and pyrite (FeS 2 ) with keV energy ion beam of cesium and oxygen. In the experiment, kinetic energy distributions of sputtered secondary ions (S + , Fe + , Pb + , S - ), as well as backscattered or re-sputtered primary ions (Cs + , O + , O - ), have been measured on a modified Cameca IMS-3f magnetic sector mass spectrometer for keV cesium (Cs + ) and oxygen (O 2 + , O - ) bombardment of galena and pyrite. Ejection of high-energy particles, with emission energies of up to ∼40% or up to ∼60% of the bombarding energy for sputtering of the lighter component (S ± ) with cesium or oxygen, respectively, and of up to ∼40% (Cs + ) and ∼80% (O ± ) for backscattering, has been observed for PbS. The computer simulations were based on the well-known MARLOWE code. In order to model the change of the stoichiometry of the binary compounds, dynamic modification of the target composition in the near-surface region was introduced. Cs incorporation was included, and a relative enrichment of the metallic component (Pb, Fe) in the top few layers due to preferential sputtering of sulfur was allowed. The computer simulations provide information on the formation of altered layer under sputter equilibrium as well as on the energy and angular emission distributions of sputtered and backscattered particles in steady-state conditions. Multiple scattering of Cs projectiles and dynamic re-sputtering of cesium that was previously incorporated in the altered near-surface region can be distinguished in the simulation, and matched with the experimental observations. In addition

Efficiency in the avail (by Com) of zinc (65ZnCl2) and phosphorus (Na H2 PO4) ions

International Nuclear Information System (INIS)

Calvache, Marcelo.

1994-01-01

The efficiency of corn to use phosphorus and zinc ions at different growing periods was determined in two soils Udic Eutrandept and Andic Haplustoll of Pichincha Province, after adding 10 ppm zinc labelled with 65Zn (gamma emisor, 1.115 meV), 50 and 100 ppm phosphorus, and a complementary fertilization. Root, stem and leaf samples were analyzed at 15 days intervals during the growing period. Zinc efficiency use was determined by isotopic method, and phosphorus by the non-isotopic. Significant differences were found for sampling period and soil types. The efficiency of use of zinc and phosphorus fertilizer increased with the age of the crop, being higher for the soil originally containing less Zn and P. Dry matter content increased linearly with phosphorus fertilizer addition

High energy argon ion irradiations of polycrystalline iron

International Nuclear Information System (INIS)

Dunlop, A.; Lesueur, D.; Lorenzelli, N.; Boulanger, L.

1986-09-01

We present here the results of our recent irradiations of polycrystalline iron targets with very energetic (1.76 GeV) Ar ions. The targets consist of piles of thin iron samples, the total thickness of each target being somewhat greater than the theoretical range (450 μm) of the ions. We can thus separate the phenomena which occur at different average energies of the ions and study during the slowing-down process: the different types of induced nuclear reactions. They allow us to determine the experimental range of the ions, the defect profiles in the targets, the structure of the displacement cascades (electron microscopy) and their stability

Characterization of phosphorus segregation in neutron-irradiated Russian pressure vessel steel weld

International Nuclear Information System (INIS)

Miller, M.K.; Jayaram, R.; Russell, K.F.

1995-01-01

An atom probe field ion microscopy characterization of three Russian pressure vessel steels has been performed. Field ion micrographs of several lath boundaries have indicated that they are decorated with a semicontinuous film of discrete brightly-imaging precipitates that were identified as molybdenum carbonitrides. In addition, extremely high phosphorus levels were measured at the lath boundaries. The phosphorus was found to be confined to an extremely narrow region indicative of monolayer type segregation. The phosphorus coverage determined from the atom probe results of the unirradiated materials agree with predictions based on McLean's equilibrium model of grain boundary segregation. The boundary phosphorus coverage of a neutron-irradiated weld material was significantly higher than in the unirradiated material. Ultrafine darkly-imaging copper- and phosphorus-enriched precipitates were also observed in the matrix of the neutron-irradiated material. (orig.)

Yolk-shell structured Sb@C anodes for high energy Na-ion batteries

Energy Technology Data Exchange (ETDEWEB)

Song, Junhua; Yan, Pengfei; Luo, Langli; Qi, Xingguo; Rong, Xiaohui; Zheng, Jianming; Xiao, Biwei; Feng, Shuo; Wang, Chongmin; Hu, Yong-Sheng; Lin, Yuehe; Sprenkle, Vincent L.; Li, Xiaolin

2017-10-01

Despite great advances in sodium-ion battery developments, the search for high energy and stable anode materials remains a challenge. Alloy or conversion-typed anode materials are attractive candidates of high specific capacity and low voltage potential, yet their applications are hampered by the large volume expansion and hence poor electrochemical reversibility and fast capacity fade. Here, we use antimony (Sb) as an example to demonstrate the use of yolk-shell structured anodes for high energy Na-ion batteries. The Sb@C yolk-shell structure prepared by controlled reduction and selective removal of Sb2O3 from carbon coated Sb2O3 nanoparticles can accommodate the Sb swelling upon sodiation and improve the structural/electrical integrity against pulverization. It delivers a high specific capacity of ~554 mAh•g-1, good rate capability (315 mhA•g-1 at 10C rate) and long cyclability (92% capacity retention over 200 cycles). Full-cells of O3-Na0.9[Cu0.22Fe0.30Mn0.48]O2 cathodes and Sb@C-hard carbon composite anodes demonstrate a high specific energy of ~130 Wh•kg-1 (based on the total mass of cathode and anode) in the voltage range of 2.0-4.0 V, ~1.5 times energy of full-cells with similar design using hard carbon anodes.

Discovery of hydrodynamic behavior in high energy heavy ion collisions

International Nuclear Information System (INIS)

Hamagaki, Hideki

2010-01-01

The objective of high energy heavy ion collision experiments is creating high temperature and high density states to investigate hadron matter properties in such extreme conditions. Since the start of heavy ion collision experiments with BEVALAC, knowledge of the space-time evolution of collision has become indispensable for understanding the hadronic matter properties. This problem is reviewed here from the hydrodynamics view point. Although its importance has been generally recognized since the time of BEVALAC, the hydrodynamic description has not been successful because the hydrodynamic model assuming non-viscous or small fluid had not been considered to be enough to properly describe the space-time evolution of hadron-hadron collisions until the RHIC experiments. Items of the following titles are picked up and reviewed here: Development of heavy ion accelerations; Space-time evolution of hadron collision process and hydrodynamic model; Chemical freezing and kinematical freezing, including transverse momentum spectra at proton-proton collisions and particle spectra in heavy ion collisions; Elliptical azimuthal angle anisotropy; Discovery of hydrodynamic flow at BEVALAC; Problems of incident beam dependence of v2; Elliptic azimuthal angle anisotropy at RHIC; What is it that carries the elliptic anisotropy? Discussion of attainment of thermodynamical equilibrium state at RHIC; and finally investigations of fluid properties other than azimuthal anisotropy, such as, Fluid properties probed by heavy quarks and Observing QCD fluid responses. (S. Funahashi)

SnSe/carbon nanocomposite synthesized by high energy ball milling as an anode material for sodium-ion and lithium-ion batteries

International Nuclear Information System (INIS)

Zhang, Zhian; Zhao, Xingxing; Li, Jie

2015-01-01

Graphical abstract: A homogeneous nanocomposite of SnSe and carbon black was synthesised by high energy ball milling and empolyed as an anode material for sodium-ion batteries (SIBs) and lithium-ion batteries (LIBs). The nanocomposite anode exhibits excellent electrochemical performances in both SIBs and LIBs. - Highlights: • A homogeneous nanocomposite of SnSe and carbon black was fabricated by high energy ball milling. • SnSe and carbon black are homogeneously mixed at the nanoscale level. • The SnSe/C anode exhibits excellent electrochemical performances in both SIBs and LIBs. - Abstract: A homogeneous nanocomposite of SnSe and carbon black, denoted as SnSe/C nanocomposite, was fabricated by high energy ball milling and empolyed as a high performance anode material for both sodium-ion batteries and lithium-ion batteries. The X-ray diffraction patterns, scanning electron microscopy and transmission electron microscopy observations confirmed that SnSe in SnSe/C nanocomposite was homogeneously distributed within carbon black. The nanocomposite anode exhibited enhanced electrochemical performances including a high capacity, long cycling behavior and good rate performance in both sodium-ion batteries (SIBs) and lithium-ion batteries (LIBs). In SIBs, an initial capacitiy of 748.5 mAh g −1 was obtained and was maintained well on cycling (324.9 mAh g −1 at a high current density of 500 mA g −1 in the 200 th cycle) with 72.5% retention of second cycle capacity (447.7 mAh g −1 ). In LIBs, high initial capacities of approximately 1097.6 mAh g −1 was obtained, and this reduced to 633.1 mAh g −1 after 100 cycles at 500 mA g −1

Limitations to depth resolution in high-energy, heavy-ion elastic recoil detection analysis

International Nuclear Information System (INIS)

Elliman, R.G.; Palmer, G.R.; Ophel, T.R.; Timmers, H.

1998-01-01

The depth resolution of heavy-ion elastic recoil detection analysis was examined for Al and Co thin films ranging in thickness from 100 to 400 nm. Measurements were performed with 154 MeV Au ions as the incident beam, and recoils were detected using a gas ionisation detector. Energy spectra were extracted for the Al and Co recoils and the depth resolution determined as a function of film thickness from the width of the high- and low- energy edges. These results were compared with theoretical estimates calculated using the computer program DEPTH. (authors)

High-energy elastic recoil detection heavy ions for light element analysis

International Nuclear Information System (INIS)

Goppelt-Langer, P.; Yamamoto, S.; Takeshita, H.; Aoki, Y.; Naramoto, H.

1994-01-01

The detection of light and medium heavy elements in not homogeneous solids is a severe problem in ion beam analysis. Heavy elements can be detected by the well established Rutherford backscattering technique (RBS). In a homogeneous host material most impurities can be easily analyzed by secondary ion mass spectroscopy (SIMS). Some isotopes ( 3 He, 6 Li, 10 B) can be measured by nuclear reaction analysis (NRA) using thermal neutrons inducing (n, p) or (n, α) reactions. Others can be detected by energetic ion beams by nuclear reactions (e.g. 15 N( 1 H, αγ) 12 C for analysis of hydrogen). A high content of H, D or T can be also determined by elastic recoil detection using an energetic He beam. The latter technique has been developed to a universal method for detection of light and heavy elements in any target, using a high energetic heavy ion beam and a detector system, which is able to identify the recoils and delivers energy and position of the particles. (author)

Charged Particle, Photon Multiplicity, and Transverse Energy Production in High-Energy Heavy-Ion Collisions

Directory of Open Access Journals (Sweden)

Raghunath Sahoo

2015-01-01

Full Text Available We review the charged particle and photon multiplicities and transverse energy production in heavy-ion collisions starting from few GeV to TeV energies. The experimental results of pseudorapidity distribution of charged particles and photons at different collision energies and centralities are discussed. We also discuss the hypothesis of limiting fragmentation and expansion dynamics using the Landau hydrodynamics and the underlying physics. Meanwhile, we present the estimation of initial energy density multiplied with formation time as a function of different collision energies and centralities. In the end, the transverse energy per charged particle in connection with the chemical freeze-out criteria is discussed. We invoke various models and phenomenological arguments to interpret and characterize the fireball created in heavy-ion collisions. This review overall provides a scope to understand the heavy-ion collision data and a possible formation of a deconfined phase of partons via the global observables like charged particles, photons, and the transverse energy measurement.

Radial transport of high-energy oxygen ions into the deep inner magnetosphere observed by Van Allen Probes

Science.gov (United States)

Mitani, K.; Seki, K.; Keika, K.; Gkioulidou, M.; Lanzerotti, L. J.; Mitchell, D. G.; Kletzing, C.

2017-12-01

It is known that proton is main contributor of the ring current and oxygen ions can make significant contribution during major magnetic storms. Ions are supplied to the ring current by radial transport from the plasma sheet. Convective transport of lower-energy protons and diffusive transport of higher-energy protons were reported to contribute to the storm-time and quiet-time ring current respectively [e.g., Gkioulidou et al., 2016]. However, supply mechanisms of the oxygen ions are not clear. To characterize the supply of oxygen ions to the ring current during magnetic storms, we studied the properties of energetic proton and oxygen ion phase space densities (PSDs) for specific magnetic moment (μ) during the April 23-25, 2013, geomagnetic storm observed by the Van Allen Probes mission. We here report on radial transport of high-energy (μ ≥ 0.5 keV/nT) oxygen ions into the deep inner magnetosphere during the late main phase of the magnetic storm. Since protons show little change during this period, this oxygen radial transport is inferred to cause the development of the late main phase. Enhancement of poloidal magnetic fluctuations is simultaneously observed. We estimated azimuthal mode number ≤5 by using cross wavelet analysis with ground-based observation of IMAGE ground magnetometers. The fluctuations can resonate with drift and bounce motions of the oxygen ions. The results suggest that combination of the drift and drift-bounce resonances is responsible for the radial transport of high-energy oxygen ions into the deep inner magnetosphere. We also report on the radial transport of the high-energy oxygen ions into the deep inner magnetosphere during other magnetic storms.

Prototype drift chamber for high energy heavy ions with a large dynamic range

International Nuclear Information System (INIS)

Kobayashi, T.; Bieser, F.; Crawford, H.; Lindstrom, P.; Baumgartner, M.; Greiner, D.

1985-01-01

The authors have constructed and tested a small prototype drift chamber designed for high energy heavy ions. When a drift chamber is used as a tracking detector for heavy projectile fragments from high energy nucleus-nucleus reactions, the major problem comes from the many spurious hits due to delta-rays. Three methods have been developed to solve this problem. The first one is to use a constant fraction discriminator to pick up the timing signal from the core ionization under the large background of delta-rays. The second one is to use pulse height information from the drift chamber to find the cell hit by the heavy ion. The last one is the idea of distributed planes. Modular planes (12 in this case) are distributed 10 cm apart on a rigid base plate to provide accurate relative positioning of the wires. The performance of the prototype chamber has been measured as a function of the high voltage bias and of the charge of the heavy ion from protons up to uranium at around 1 GeV/nucleon

Radiation effects on semiconductor devices in high energy heavy ion accelerators

Energy Technology Data Exchange (ETDEWEB)

Belousov, Anton

2014-10-20

Radiation effects on semiconductor devices in GSI Helmholtz Center for Heavy Ion Research are becoming more and more significant with the increase of beam intensity due to upgrades. Moreover a new accelerator is being constructed on the basis of GSI within the project of facility for antiproton and ion research (FAIR). Beam intensities will be increased by factor of 100 and energies by factor of 10. Radiation fields in the vicinity of beam lines will increase more than 2 orders of magnitude and so will the effects on semiconductor devices. It is necessary to carry out a study of radiation effects on semiconductor devices considering specific properties of radiation typical for high energy heavy ion accelerators. Radiation effects on electronics in accelerator environment may be divided into two categories: short-term temporary effects and long-term permanent degradation. Both may become critical for proper operation of some electronic devices. This study is focused on radiation damage to CCD cameras in radiation environment of heavy ion accelerator. Series of experiments with irradiation of devices under test (DUTs) by secondary particles produced during ion beam losses were done for this study. Monte Carlo calculations were performed to simulate the experiment conditions and conditions expected in future accelerator. Corresponding comparisons and conclusions were done. Another device typical for accelerator facilities - industrial Ethernet switch was tested in similar conditions during this study. Series of direct irradiations of CCD and MOS transistors with heavy ion beams were done as well. Typical energies of the primary ion beams were 0.5-1 GeV/u. Ion species: from Na to U. Intensities of the beam up to 10{sup 9} ions/spill with spill length of 200-300 ns. Criteria of reliability and lifetime of DUTs in specific radiation conditions were formulated, basing on experimental results of the study. Predictions of electronic device reliability and lifetime were

Comparative study between hadron and heavy ion dissociation at high energies

International Nuclear Information System (INIS)

El-Bakry, Y.M.N.; Abd-Elhalim, S.M.

2002-01-01

The present work deals with the dissociation of hadrons and heavy ions at high energies. In investigating hadron nucleus and nucleus-nucleus collisions, it is important to classify the experimental data, into two main classes; the coherent. and incoherent reactions. The coherent production is the main of our study. This process called electromagnetic dissociation (ED) and can be differentiate into coulomb dissociation (CD) and diffraction dissociation (DD). This work explains the experimental data of collisions of hadrons K± (70 GeV/c) and π(340 Gc V/c) and heavy ions 6 L i, 7 L i, 1 2C and1 6O at Dubna energies (3-4.5 A GeV/c)with emulsion target, in the frame of some models and theories which describe the mechanism of ED dissociation

Exploring resource efficiency for energy, land and phosphorus use

NARCIS (Netherlands)

Berg, van den Maurits; Hermans, Kathleen; Vuuren, van Detlef P.; Bouwman, A.F.; Kram, Tom; Bakkes, Jan

2016-01-01

In this paper, we present four model-based scenarios exploring the potential for resource efficiency for energy, land and phosphorus use, and implications for resource depletion, climate change and biodiversity. The scenarios explored include technological improvements as well as structural

Damage of plasmid DNA by high energy ions

International Nuclear Information System (INIS)

Michaelidesova, A.; Pachnerova Brabcova, K.; Davidkova, M.

2018-01-01

The aim of the study was to determine the degree of direct DNA damage by high-energy ions, which are one of the components of cosmic rays, and therefore the knowledge of the biological effects of these ions is key to long-term space missions with human crew. The pBR322 plasmid containing 4361 base pairs was used in this study. The aqueous solution of plasmid pBR322 was transferred on ice to Japan to the Heavy Ion Medical Accelerator in Chiba, the Research Center for Charged Particle Therapy. Just before the experiment, the droplets of solution of known concentration were applied to the slides and the water was allowed to evaporate to produce dry DNA samples. Half of the slides were irradiated with 290 MeV/u of carbon ions and a dose rate of 20 Gy/min. The other half of the slides were irradiated with helium nuclei of 150 MeV/hr and a dose rate of 12.6 Gy/min. Both sets of slides were irradiated with doses of 0-1,400 Gy with a 200 Gy step. After irradiation, the samples were re-dissolved in distilled water, frozen and transported on ice to the Czech Republic for processing. Samples were analyzed by agarose gel electrophoresis. The plasmid was evaluated separately to determine the degree of radiation induced lesions and further to incubation with enzymes recognizing basal damage. (authors)

Nitrogen-Doped Carbon for Red Phosphorous Based Anode Materials for Lithium Ion Batteries

Directory of Open Access Journals (Sweden)

Jiaoyang Li

2018-01-01

Full Text Available Serving as conductive matrix and stress buffer, the carbon matrix plays a pivotal role in enabling red phosphorus to be a promising anode material for high capacity lithium ion batteries and sodium ion batteries. In this paper, nitrogen-doping is proved to effective enhance the interface interaction between carbon and red phosphorus. In detail, the adsorption energy between phosphorus atoms and oxygen-containing functional groups on the carbon is significantly reduced by nitrogen doping, as verified by X-ray photoelectron spectroscopy. The adsorption mechanisms are further revealed on the basis of DFT (the first density functional theory calculations. The RPNC (red phosphorus/nitrogen-doped carbon composite material shows higher cycling stability and higher capacity than that of RPC (red phosphorus/carbon composite anode. After 100 cycles, the RPNC still keeps discharge capacity of 1453 mAh g−1 at the current density of 300 mA g−1 (the discharge capacity of RPC after 100 cycles is 1348 mAh g−1. Even at 1200 mA g−1, the RPNC composite still delivers a capacity of 1178 mAh g−1. This work provides insight information about the interface interactions between composite materials, as well as new technology develops high performance phosphorus based anode materials.

High performance of nitrogen and phosphorus removal in an electrolysis-integrated biofilter.

Science.gov (United States)

Gao, Y; Xie, Y W; Zhang, Q; Yu, Y X; Yang, L Y

A novel electrolysis-integrated biofilter system was developed in this study to evaluate the intensified removal of nitrogen and phosphorus from contaminated water. Two laboratory-scale biofilter systems were established, one with electrolysis (E-BF) and one without electrolysis (BF) as control. The dynamics of intensified nitrogen and phosphorus removal and the changes of inflow and outflow water qualities were also evaluated. The total nitrogen (TN) removal rate was 94.4% in our newly developed E-BF, but only 74.7% in the control BF. Ammonium removal rate was up to 95% in biofilters with or without electrolysis integration with an influent ammonium concentration of 40 mg/L, and the accumulation of nitrate and nitrite was much lower in the effluent of E-BF than that of BF. Thus electrolysis plays an important role in TN removal especially the nitrate and nitrite removal. Phosphorus removal was significantly enhanced, exceeding 90% in E-BF by chemical precipitation, physical adsorption, and flocculation of phosphorus because of the in situ formation of ferric ions by the anodizing of sacrificial iron anodes. Results from this study indicate that the electrolysis integrated biofilter is a promising solution for intensified nitrogen and phosphorus removal.

High-energy ion-beam-induced phase separation in SiOx films

International Nuclear Information System (INIS)

Arnoldbik, W.M.; Tomozeiu, N.; Hattum, E.D. van; Lof, R.W.; Vredenberg, A.M.; Habraken, F.H.P.M.

2005-01-01

The modification of the nanostructure of silicon suboxide (SiO x ) films as a result of high-energy heavy-ion irradiation has been studied for the entire range 0.1≤x x films have been obtained by radio-frequency magnetron sputter deposition. For 50 MeV 63 Cu 8+ ions and an angle of incidence of 20 deg. with the plane of the surface, and for x≥0.5, it takes a fluence of about 10 14 /cm 2 to reach a Si-O-Si infrared absorption spectrum, which is supposed to be characteristic for a Si-SiO 2 composite film structure. For smaller x values, it takes a much larger fluence. The interpretation of the IR spectra is corroborated for the surface region by results from x-ray photoelectron spectroscopy. The results present evidence for a mechanism, in which the phase separation takes place in the thermal spike, initiated by the energy deposited in many overlapping independent ion tracks. Such a process is possible since the suboxides fulfill the conditions for spinodal decomposition

The influence of phosphorus on the corrosion of iron in calcium nitrate

International Nuclear Information System (INIS)

Windisch, C.F. Jr.; Baer, D.R.; Jones, R.H.; Engelhard, M.H.

1992-01-01

This paper reports that intergranular stress corrosion cracking (IGSCC) of metallic alloys including iron is strongly influenced by the presence of grain boundary impurities such as phosphorus. In this study to determine how phosphorus affects the corrosion of ion, electrochemical polarization methods were used in conjunction with surface analyses employing ultrahigh vacuum transfer. Specifically, these methods were used to examine the corrosion of iron, iron/phosphorus alloys, and iron implanted with phosphorus in deaerated 55 weight percent Ca(NO 3 ) 2 solutions at 60 degrees C. The presence of phosphorus in iron accelerated corrosion in both the active and passive regions, with the effect being more pronounced in the passive region. In the active region, the phosphorus was oxidized to phosphate which, in turn, appeared to assist the dissolution of the semiprotective Fe 3 O 4 . In the passive region, the phosphorus (when unoxidized) accelerated corrosion by some other mechanism. The FePO 4 that formed in the passive region did not inhibit passivation by, rather, was incorporated in the passive film. The chemical transformations would appear to explain, at least partly, the high IGSCC rates observed for ion containing phosphorus segregated at grain boundaries

Measurements of the Properties of Highly-charged high-Z ions

International Nuclear Information System (INIS)

Augustine J. Smith, Ph.D.

2007-01-01

We had proposed carrying out a systematic experimental investigation of the atomic physics of highly charged, high-Z ions, produced in the Lawrence Livermore National Laboratory LLNL electron beam ion trap (EBIT-I) in its high energy mode, superEBIT. In particular we were going to accurately measure line positions for Δn=0 transitions in few electron high-Z ions; this was meant to enable us to investigate relativistic and quantum electrodynamics QED contributions to the energy levels as well as the nuclear properties of heavy ions. We were also going to measure cross sections for various electron-ion interactions, the degree of polarization of emitted x-rays, and radiation cooling rates of various ionization stages of highly charged, high-Z ions. This would enable us to study fundamental atomic physics of high-Z ions at relativistic electron impact energies and in the intense nuclear fields of highly ionized, high-Z ions. This would extend previous measurements we have carried out to a regime where there is a paucity of good data. These measurements were expected to generate increased theoretical interest and activity in this area. The project will extend a very successful collaboration between Morehouse College (MC) and a national laboratory LLNL, Minority student training and development are major components of the proposal

Soft errors in 10-nm-scale magnetic tunnel junctions exposed to high-energy heavy-ion radiation

Science.gov (United States)

Kobayashi, Daisuke; Hirose, Kazuyuki; Makino, Takahiro; Onoda, Shinobu; Ohshima, Takeshi; Ikeda, Shoji; Sato, Hideo; Inocencio Enobio, Eli Christopher; Endoh, Tetsuo; Ohno, Hideo

2017-08-01

The influences of various types of high-energy heavy-ion radiation on 10-nm-scale CoFeB-MgO magnetic tunnel junctions with a perpendicular easy axis have been investigated. In addition to possible latent damage, which has already been pointed out in previous studies, high-energy heavy-ion bombardments demonstrated that the magnetic tunnel junctions may exhibit clear flips between their high- and low-resistance states designed for a digital bit 1 or 0. It was also demonstrated that flipped magnetic tunnel junctions still may provide proper memory functions such as read, write, and hold capabilities. These two findings proved that high-energy heavy ions can produce recoverable bit flips in magnetic tunnel junctions, i.e., soft errors. Data analyses suggested that the resistance flips stem from magnetization reversals of the ferromagnetic layers and that each of them is caused by a single strike of heavy ions. It was concurrently found that an ion strike does not always result in a flip, suggesting a stochastic process behind the flip. Experimental data also showed that the flip phenomenon is dependent on the device and heavy-ion characteristics. Among them, the diameter of the device and the linear energy transfer of the heavy ions were revealed as the key parameters. From their dependences, the physical mechanism behind the flip was discussed. It is likely that a 10-nm-scale ferromagnetic disk loses its magnetization due to a local temperature increase induced by a single strike of heavy ions; this demagnetization is followed by a cooling period associated with a possible stochastic recovery process. On the basis of this hypothesis, a simple analytical model was developed, and it was found that the model accounts for the results reasonably well. This model also predicted that magnetic tunnel junctions provide sufficiently high soft-error reliability for use in space, highlighting their advantage over their counterpart conventional semiconductor memories.

Study of high energy ion implantation of boron and oxygen in silicon

International Nuclear Information System (INIS)

Thevenin, P.

1991-06-01

Three aspects of high energy (0.5-3 MeV) light ions ( 11 B + and 16 O + ) implantation in silicon are examined: (1)Spatial repartition; (2) Target damage and (3) Synthesis by oxygen implantation of a buried silicon oxide layer

Magnetized retarding field energy analyzer measuring the particle flux and ion energy distribution of both positive and negative ions

International Nuclear Information System (INIS)

Rafalskyi, Dmytro; Aanesland, Ane; Dudin, Stanislav

2015-01-01

This paper presents the development of a magnetized retarding field energy analyzer (MRFEA) used for positive and negative ion analysis. The two-stage analyzer combines a magnetic electron barrier and an electrostatic ion energy barrier allowing both positive and negative ions to be analyzed without the influence of electrons (co-extracted or created downstream). An optimal design of the MRFEA for ion-ion beams has been achieved by a comparative study of three different MRFEA configurations, and from this, scaling laws of an optimal magnetic field strength and topology have been deduced. The optimal design consists of a uniform magnetic field barrier created in a rectangular channel and an electrostatic barrier consisting of a single grid and a collector placed behind the magnetic field. The magnetic barrier alone provides an electron suppression ratio inside the analyzer of up to 6000, while keeping the ion energy resolution below 5 eV. The effective ion transparency combining the magnetic and electrostatic sections of the MRFEA is measured as a function of the ion energy. It is found that the ion transparency of the magnetic barrier increases almost linearly with increasing ion energy in the low-energy range (below 200 eV) and saturates at high ion energies. The ion transparency of the electrostatic section is almost constant and close to the optical transparency of the entrance grid. We show here that the MRFEA can provide both accurate ion flux and ion energy distribution measurements in various experimental setups with ion beams or plasmas run at low pressure and with ion energies above 10 eV

Advanced Nanostructured Cathode for Ultra High Specific Energy Lithium Ion Batteries, Phase I

Data.gov (United States)

National Aeronautics and Space Administration — Integrate advanced nanotechnology with energy storage technology to develop advanced cathode materials for use in Li-ion batteries while maintaining a high level of...

Applications of high energy neutralized ion beams to a compact torus

International Nuclear Information System (INIS)

Rostoker, N.; Katzenstein, J.

1986-01-01

Pulsed ion beams can be produced with ion diodes and Marx generators. The technology exists to produce high energy beams efficiently. A neutralized ion beam has an equal number of co-moving electrons. The resultant beam is electrically neutral, has no net current and can be transported across a magnetic field if the current density is sufficiently large. Preliminary experimental results have been obtained on injecting a neutralized proton beam into a small tokamak. To illuminate the physical processes involved in injection and trapping an experiment has been designed for TEXT. Possible applications to a compact torus include plasma heating, current maintenance and non-equilibrium reactors that do not require ignition. Each application is discussed and comparisons are made with other methods. (author)

Heavy ion scattering: High energy limits of RBS and ERD

International Nuclear Information System (INIS)

Rauhala, E.

1994-01-01

Elastic scattering of 7 Li ions by oxygen and 12 C, 14 N and 16 O ions by aluminum, silicon, titanium and sulfur have been studied below the Coulomb barrier energies 3-30 MeV in the angular range of 78 degrees - 170 degrees. By kinematically reversing the reactions, the recoiling of carbon, nitrogen and oxygen by 40-100 MeV 27 Al, 28 Si, 32S and 48 Ti ions into recoil angles of 20 degrees, 25 degrees, 30 degrees and 40 degrees has also been investigated. Excitation functions and angular distributions are presented. Contrary to the case of light H and He ions, the heavy ion scattering cross sections fall off rapidly above the non-Rutherford threshold energy, rendering heavy ion RBS and ERD spectrometry worthless. Both classical and wave mechanical calculations have been attempted for predicting the RBS threshold energies. Simple calculations give moderate accuracy, while the more extensive nuclear potential perturbation approach relies on parameters fitted for the particular experiment. The authors present a general classical semi-empirical model for both direct scattering (RBS) and the kinematically reversed reactions (ERD), accurately reproducing the experimental data. The model is based on parameters fitted from the present scattering experiments and from an extensive literature survey

Low Li+ Insertion Barrier Carbon for High Energy Efficient Lithium-Ion Capacitor.

Science.gov (United States)

Lee, Wee Siang Vincent; Huang, Xiaolei; Tan, Teck Leong; Xue, Jun Min

2018-01-17

Lithium-ion capacitor (LIC) is an attractive energy-storage device (ESD) that promises high energy density at moderate power density. However, the key challenge in its design is the low energy efficient negative electrode, which barred the realization of such research system in fulfilling the current ESD technological inadequacy due to its poor overall energy efficiency. Large voltage hysteresis is the main issue behind high energy density alloying/conversion-type materials, which reduces the electrode energy efficiency. Insertion-type material though averted in most research due to the low capacity remains to be highly favorable in commercial application due to its lower voltage hysteresis. To further reduce voltage hysteresis and increase capacity, amorphous carbon with wider interlayer spacing has been demonstrated in the simulation result to significantly reduce Li + insertion barrier. Hence, by employing such amorphous carbon, together with disordered carbon positive electrode, a high energy efficient LIC with round-trip energy efficiency of 84.3% with a maximum energy density of 133 Wh kg -1 at low power density of 210 W kg -1 can be achieved.

Ultrafast and directional diffusion of lithium in phosphorene for high-performance lithium-ion battery.

Science.gov (United States)

Li, Weifeng; Yang, Yanmei; Zhang, Gang; Zhang, Yong-Wei

2015-03-11

Density functional theory calculations have been performed to investigate the binding and diffusion behavior of Li in phosphorene. Our studies reveal the following findings: (1) Li atom forms strong binding with phosphorus atoms and exists in the cationic state; (2) the shallow energy barrier (0.08 eV) of Li diffusion on monolayer phosphorene along zigzag direction leads to an ultrahigh diffusivity, which is estimated to be 10(2) (10(4)) times faster than that on MoS2 (graphene) at room temperature; (3) the large energy barrier (0.68 eV) along armchair direction results in a nearly forbidden diffusion, and such strong diffusion anisotropy is absent in graphene and MoS2; (4) a remarkably large average voltage of 2.9 V is predicted in the phosphorene-based Li-ion battery; and (5) a semiconducting to metallic transition induced by Li intercalation of phosphorene gives rise to a good electrical conductivity, ideal for use as an electrode. Given these advantages, it is expected that phosphorene will present abundant opportunities for applications in novel electronic device and lithium-ion battery with a high rate capability and high charging voltage.

Phosphorus vacancy cluster model for phosphorus diffusion gettering of metals in Si

Energy Technology Data Exchange (ETDEWEB)

Chen, Renyu; Trzynadlowski, Bart; Dunham, Scott T. [Department of Electrical Engineering, University of Washington, Seattle, Washington 98195 (United States)

2014-02-07

In this work, we develop models for the gettering of metals in silicon by high phosphorus concentration. We first performed ab initio calculations to determine favorable configurations of complexes involving phosphorus and transition metals (Fe, Cu, Cr, Ni, Ti, Mo, and W). Our ab initio calculations found that the P{sub 4}V cluster, a vacancy surrounded by 4 nearest-neighbor phosphorus atoms, which is the most favorable inactive P species in heavily doped Si, strongly binds metals such as Cu, Cr, Ni, and Fe. Based on the calculated binding energies, we build continuum models to describe the P deactivation and Fe gettering processes with model parameters calibrated against experimental data. In contrast to previous models assuming metal-P{sub 1}V or metal-P{sub 2}V as the gettered species, the binding of metals to P{sub 4}V satisfactorily explains the experimentally observed strong gettering behavior at high phosphorus concentrations.

Scanning ion microscopy with low energy lithium ions

International Nuclear Information System (INIS)

Twedt, Kevin A.; Chen, Lei; McClelland, Jabez J.

2014-01-01

Using an ion source based on photoionization of laser-cooled lithium atoms, we have developed a scanning ion microscope with probe sizes of a few tens of nanometers and beam energies from 500 eV to 5 keV. These beam energies are much lower than the typical operating energies of the helium ion microscope or gallium focused ion beam systems. We demonstrate how low energy can be advantageous in ion microscopy when detecting backscattered ions, due to a decreased interaction volume and the potential for surface sensitive composition analysis. As an example application that demonstrates these advantages, we non-destructively image the removal of a thin residual resist layer during plasma etching in a nano-imprint lithography process. - Highlights: • We use an ion source based on photoionization of laser-cooled lithium atoms. • The ion source makes possible a low energy (500 eV to 5 keV) scanning ion microscope. • Low energy is preferred for ion microscopy with backscattered ions. • We use the microscope to image a thin resist used in nano-imprint lithography

A highly sensitive CaF{sub 2}:Dy nanophosphor as an efficient low energy ion dosimetry

Energy Technology Data Exchange (ETDEWEB)

Bhadane, Mahesh S.; Hareesh, K.; Dahiwale, S.S.; Sature, K.R. [Microtron Accelerator Laboratory, Department of Physics, Savitribai Phule Pune University, Pune 411007 (India); Patil, B.J. [Department of Physics, Abasaheb Garware College, Pune 411004 (India); Asokan, K.; Kanjilal, D. [Inter University Accelerator Centre, Aruna Asaf Ali Marg, New Delhi 110067 (India); Bhoraskar, V.N. [Microtron Accelerator Laboratory, Department of Physics, Savitribai Phule Pune University, Pune 411007 (India); Dhole, S.D., E-mail: sanjay@physics.unipune.ac.in [Microtron Accelerator Laboratory, Department of Physics, Savitribai Phule Pune University, Pune 411007 (India)

2016-11-01

Highlights: • CaF{sub 2}:Dy nanophosphor synthesized by chemical co-precipitation route. • Phosphors are irradiated by H, Ar and N low energy ions at different fluences. • LEBI irradiated phosphors are characterized by XRD, TEM, FTIR and PL spectroscopy. • First time report to LEIB irradiated for thermoluminescence dosimetric applications. - Abstract: Dysprosium doped calcium fluoride (CaF{sub 2}:Dy) powers synthesized by co-precipitation method were irradiated with low energy ion beams (LEIB) viz. 100 keV H, 200 keV Ar and 350 keV N beams at different fluences and demonstrated for low energy ion dosimetric application. X-ray Diffraction and Transmission electron microscopy revealed the formation of highly crystalline cubic structured particles with size ∼45–50 nm. FTIR spectra of the CaF{sub 2}:Dy samples show changes of some bonds such as N–O asymmetric, C–F bonding and C–H aromatic contain stretching mode after LEIB irradiation. The thermoluminescence (TL) glow curve peaks were observed at 207 °C for Ar ion, at 203 °C for H ion and at 216 °C and 270 °C for N ion. It has been found that CaF{sub 2}:Dy nanophosphor shows a linear response with minimum fading for all the ion species. Computerized Glow Curve Deconvolution was performed for TL curve of high fluence ion irradiated nanophosphor to estimate the trapping parameters and the respective figure of merit (FOM) found to be very appropriate for all the nanophosphor. These results indicated that the CaF{sub 2}:Dy can be used as a low energy ion detector or dose.

Lamb-shift measurement in hydrogenic phosphorus

International Nuclear Information System (INIS)

Pross, H.; Budelsky, D.; Kremer, L.; Platte, D.; von Brentano, P.; Gassen, J.; Mueller, D.; Scheuer, F.; Pape, A.; Sens, J.C.

1993-01-01

The final result of a 2s 2 S 1/2-- 2p 2 P 1/2 Lamb-shift measurement by the laser resonance method in hydrogenic phosphorus is reported. Metastable 2s 2 S 1/2 ions were prepared using a β∼0.08 velocity beam of 31 P 14+ ions obtained from the MP tandem accelerator at the Centre de Recherches Nucleaires in Strasbourg. From the metastable state the transition to the 2p 2 P 3/2 state was induced with a high-power dye laser leading to a measured transition energy of ΔE=2.231 33(12) eV. Subtracting the well-known fine-structure splitting ΔE FS =2.314 82(2) eV, the Lamb shift is deduced to be E expt (LS)=20 188(29) GHz. This result is compared with the theoretical value E theor (LS)=20 254(10) GHz and with other experimental results for the Lamb shift in the region Z≤18. Finally, the utility of the Lamb-shift measurements in testing the G(Zα) function of the self-energy, which includes only terms in (Zα) n , n≥6, is discussed

Thermal spike analysis of highly charged ion tracks

International Nuclear Information System (INIS)

Karlušić, M.; Jakšić, M.

2012-01-01

The irradiation of material using swift heavy ion or highly charged ion causes excitation of the electron subsystem at nanometer scale along the ion trajectory. According to the thermal spike model, energy deposited into the electron subsystem leads to temperature increase due to electron–phonon coupling. If ion-induced excitation is sufficiently intensive, then melting of the material can occur, and permanent damage (i.e., ion track) can be formed upon rapid cooling. We present an extension of the analytical thermal spike model of Szenes for the analysis of surface ion track produced after the impact of highly charged ion. By applying the model to existing experimental data, more than 60% of the potential energy of the highly charged ion was shown to be retained in the material during the impact and transformed into the energy of the thermal spike. This value is much higher than 20–40% of the transferred energy into the thermal spike by swift heavy ion. Thresholds for formation of highly charged ion track in different materials show uniform behavior depending only on few material parameters.

Investigation of the energy loss and the charge state of high energy heavy ions in a hydrogen plasma

International Nuclear Information System (INIS)

Dietrich, K.G.

1991-07-01

For heavy ions with energy of 1.4 to 5.9 MeV/u the energy loss and charge state after transmission through a totally ionized hydrogen plasma are investigated. Plasma target was a Z-pinch device incorporated in the beam optics of the accelerator by a pumping system. In the 20 cm long pinch hydrogen plasmas with densities up to 1.5x10 19 cm -3 and temperatures above 5 eV are produced, with ionization efficiency higher than 99%. The ions pass the plasma on the symmetry axis of the plasma column through small apertures in the electrodes. The energy loss was measured by time-of-flight method, the plasma density by interferometry along the pinch axis. For the first time the ion charge after transmission through the plasma has been determined by a charge spectrometer being a combination of a dipole magnet and a position sensitive detector with high time resolution. A growth of the average charge of heavy ions in plasma higher than the equilibrium charge in cold gas was discovered, caused by a reduction of electron capture by fast heavy ions in ionized matter. The electron loss rates in plasma and cold gas are equal. (orig./AH) [de

Deep level transient spectroscopy studies of charge traps introduced into silicon by channeling ion implantation of phosphorus

International Nuclear Information System (INIS)

McCallum, J.C.; Lay, M.; Deenapanray, P.N.K.; Jagadish, C.

2002-01-01

Full text: The operating conditions of a silicon-based quantum computer are expected to place stringent requirements on the quality of the material and the processes used to make it. In the Special Research Centre for Quantum Computer Technology, ion implantation is one of the principle processing techniques under investigation for forming an ordered array of phosphorus atoms. This technique introduces defect centres in silicon which act as charge traps. Charge traps are expected to be detrimental to operation of the device. These defect centres, their dependence on ion implantation and thermal annealing conditions are being quantified using Deep Level Transient Spectroscopy (DLTS). Since the aspect ratio of the masks required for the top-down fabrication process restrict the incident ions to a range of angles in which they may undergo channeling implantation in the silicon substrate, we have examined the effect of channeling implantation on the nature and quantity of the charge traps produced. This is the first time that DLTS studies have been performed for channeling implantation of a dopant species in silicon. DLTS is well-suited to the dose regime of ∼10 11 P/cm 3 required for the quantum computer, however, a standard DLTS measurement is unable to probe the shallow depth range of ∼ 20 nm required for the P atoms (∼ 10-15 keV implantation energy). Our aim has therefore been to perform P implants in the appropriate dose regime but using higher implantation energies, ∼ 75-450 keV, where DLTS can directly identify and profile the charge traps induced by the implantation step and monitor their annealing characteristics during subsequent processing. To map the behaviour observed in this energy regime onto the low energy range required for the quantum computer we are comparing the DLTS results to damage profiles predicted by the Monte Carlo code Crystal Trim which is used in the semiconductor industry to simulate ion implantation processes in crystalline

Chromatography of phosphorus oxoacids

International Nuclear Information System (INIS)

Ohashi, S.

1975-01-01

The present state of studies on the chromatographic separation of phosphorus oxoacids is surveyed. In this paper, chromatographic techniques are divided into four groups, i.e. paper and thin-layer chromatography, paper electrophoresis, ion-exchange chromatography, and gel chromatography. The separation mechanisms and characteristics for these chromatographic methods are discussed and some examples for the separation of phosphorus oxoacids are described. As examples of the application of ion-exchange and gel chromatography, studies on the hot atom chemistry of 32 P in solid inorganic phosphates and those on the substitution reactions between diphosphonate (diphosphite) and polyphosphates are reported. (author)

Quantitative evaluation of high-energy O- ion particle flux in a DC magnetron sputter plasma with an indium-tin-oxide target

Science.gov (United States)

Suyama, Taku; Bae, Hansin; Setaka, Kenta; Ogawa, Hayato; Fukuoka, Yushi; Suzuki, Haruka; Toyoda, Hirotaka

2017-11-01

O- ion flux from the indium tin oxide (ITO) sputter target under Ar ion bombardment is quantitatively evaluated using a calorimetry method. Using a mass spectrometer with an energy analyzer, O- energy distribution is measured with spatial dependence. Directional high-energy O- ion ejected from the target surface is observed. Using a calorimetry method, localized heat flux originated from high-energy O- ion is measured. From absolute evaluation of the heat flux from O- ion, O- particle flux in order of 1018 m-2 s-1 is evaluated at a distance of 10 cm from the target. Production yield of O- ion on the ITO target by one Ar+ ion impingement at a kinetic energy of 244 eV is estimated to be 3.3  ×  10-3 as the minimum value.

Chemical modifications of polymer films induced by high energy heavy ions

International Nuclear Information System (INIS)

Zhu Zhiyong; Sun Youmei; Liu Changlong; Liu Jie; Jin Yunfan

2002-01-01

Polymer films including polyethylene terephthalate (PET), polystyrene (PS) and polycarbonate (PC) were irradiated at room temperature with ions of 35 MeV/u 40 Ar, 25 MeV/u 84 Kr, 15.1 MeV/u 136 Xe and 11.4 MeV/u 238 U to fluences ranging from 9x10 9 to 5.5x10 12 ions/cm 2 . The radiation-induced chemical changes of the materials were investigated by Fourier-transform infrared (FTIR) and ultraviolet/visible spectroscopies. It is found that the absorbance in the ultraviolet and visible range induced by all irradiations follows a linear relationship with fluence. The radiation-induced absorbance normalized to one particle increases slowly with increasing of electronic energy loss below about 8 keV/nm followed by a sharp increase up to about 15 keV/nm above which saturation is reached. FTIR measurements reveal that the materials suffer serious degradation through bond breaking. The absorbance of the typical infrared bands decays exponentially with increase of ion fluence and the bond-disruption cross-section shows a sigmoid variation with electronic energy loss. In PET loss of crystallinity is attributed to the configuration transformation of the ethylene glycol residue from trans into the gauche. Alkyne end groups are induced in all the materials above certain electronic energy loss threshold, which is found to be about 0.8 keV/nm for PS and 0.4 keV/nm for PC. The production cross-section of alkyne end group increases with increasing of electronic energy loss and shows saturation at high electronic energy loss values. It is concluded that not only the physical processes but also the chemical processes of the energy deposition determine the modification of polymer

Ion implantation into amorphous Si layers to form carrier-selective contacts for Si solar cells

International Nuclear Information System (INIS)

Feldmann, Frank; Mueller, Ralph; Reichel, Christian; Hermle, Martin

2014-01-01

This paper reports our findings on the boron and phosphorus doping of very thin amorphous silicon layers by low energy ion implantation. These doped layers are implemented into a so-called tunnel oxide passivated contact structure for Si solar cells. They act as carrier-selective contacts and, thereby, lead to a significant reduction of the cell's recombination current. In this paper we address the influence of ion energy and ion dose in conjunction with the obligatory high-temperature anneal needed for the realization of the passivation quality of the carrier-selective contacts. The good results on the phosphorus-doped (implied V oc = 725 mV) and boron-doped passivated contacts (iV oc = 694 mV) open a promising route to a simplified interdigitated back contact (IBC) solar cell featuring passivated contacts. (copyright 2014 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

Rechargeable dual-metal-ion batteries for advanced energy storage.

Science.gov (United States)

Yao, Hu-Rong; You, Ya; Yin, Ya-Xia; Wan, Li-Jun; Guo, Yu-Guo

2016-04-14

Energy storage devices are more important today than any time before in human history due to the increasing demand for clean and sustainable energy. Rechargeable batteries are emerging as the most efficient energy storage technology for a wide range of portable devices, grids and electronic vehicles. Future generations of batteries are required to have high gravimetric and volumetric energy, high power density, low price, long cycle life, high safety and low self-discharge properties. However, it is quite challenging to achieve the above properties simultaneously in state-of-the-art single metal ion batteries (e.g. Li-ion batteries, Na-ion batteries and Mg-ion batteries). In this contribution, hybrid-ion batteries in which various metal ions simultaneously engage to store energy are shown to provide a new perspective towards advanced energy storage: by connecting the respective advantages of different metal ion batteries they have recently attracted widespread attention due to their novel performances. The properties of hybrid-ion batteries are not simply the superposition of the performances of single ion batteries. To enable a distinct description, we only focus on dual-metal-ion batteries in this article, for which the design and the benefits are briefly discussed. We enumerate some new results about dual-metal-ion batteries and demonstrate the mechanism for improving performance based on knowledge from the literature and experiments. Although the search for hybrid-ion batteries is still at an early age, we believe that this strategy would be an excellent choice for breaking the inherent disadvantages of single ion batteries in the near future.

IMP-8 observations of the spectra, composition, and variability of solar heavy ions at high energies relevant to manned space missions

International Nuclear Information System (INIS)

Tylka, Allan J.; Dietrich, William F.

1999-01-01

In more than 25 years of almost continuous observations, the University of Chicago's Cosmic Ray Telescope (CRT) on IMP-8 has amassed a unique database on high-energy solar heavy ions of potential relevance to manned spaceflight. In the very largest particle events, IMP-8/CRT has even observed solar Fe ions above the Galactic cosmic ray background up to ∼800 MeV/nucleon, an energy sufficiently high to penetrate nearly 25 g/cm 2 of shielding. IMP-8/CRT observations show that high-energy heavy-ion spectra are often surprisingly hard power laws, without the exponential roll-offs suggested by stochastic acceleration fits to lower energy measurements alone. Also, in many solar particle events the Fe/O ratio grows with increasing energy, contrary to the notion that ions with higher mass-to-charge ratios should be less abundant at higher energies. Previous studies of radiation hazards for manned spaceflight have often assumed heavy-ion composition and steeply-falling energy spectra inconsistent with these observations. Conclusions based on such studies should therefore be re-assessed. The significant event-to-event variability observed in the high-energy solar heavy ions also has important implications for strategies in building probabilistic models of solar particle radiation hazards

phosphorus sorption capacity as a guide for phosphorus availability

African Journals Online (AJOL)

Prof. Adipala Ekwamu

drained, light yellowish brown, loamy sand ... Dongola 2 Akked series: Deep, dark grayish brown, clay ... energy. Statistical analysis. Data collected were statistically analysed using ANOVA of MStatc ... phosphorus sorbed versus phosphorus.

Production of nanodiamonds by high-energy ion irradiation of graphite at room temperature

International Nuclear Information System (INIS)

Daulton, T.L.; Kirk, M.A.; Lewis, R.S.; Rehn, L.E.

2001-01-01

It has previously been shown that graphite can be transformed into diamond by MeV electron and ion irradiation at temperatures above approximately 600 deg. C. However, there exists geological evidence suggesting that carbonaceous materials can be transformed to diamond by irradiation at substantially lower temperatures. For example, submicron-size diamond aggregates have been found in uranium-rich, Precambrian carbonaceous deposits that never experienced high temperature or pressure. To test if diamonds can be formed at lower irradiation temperatures, sheets of fine-grain polycrystalline graphite were bombarded at 20 deg. C with 350±50 MeV Kr ions to fluences of 6x10 12 cm -2 using the Argonne tandem linear accelerator system (ATLAS). Ion-irradiated (and unirradiated control) graphite specimens were then subjected to acid dissolution treatments to remove untransformed graphite and isolate diamonds that were produced; these acid residues were subsequently characterized by high-resolution and analytical electron microscopy. The acid residue of the ion-irradiated graphite was found to contain nanodiamonds, demonstrating that ion irradiation of graphite at ambient temperature can produce diamond. The diamond yield under our irradiation conditions is low, ∼0.01 diamonds/ion. An important observation that emerges from comparing the present result with previous observations of diamond formation during irradiation is that nanodiamonds form under a surprisingly wide range of irradiation conditions. This propensity may be related to the very small difference in the graphite and diamond free-energies coupled with surface-energy considerations that may alter the relative stability of diamond and graphite at nanometer sizes

Equilibrium charge state distributions of high energy heavy ions

International Nuclear Information System (INIS)

Clark, R.B.; Grant, I.S.; King, R.; Eastham, D.A.; Joy, T.

1976-01-01

Equilibrium charge state fractions have been measured for N, O, Ne, S, Ar and Kr ions at 1.04 MeV/nucleon after passing through various stripping materials. Further data were obtained at higher energy for S ions (4.12 MeV/nucleon) and Ar ions (4.12 and 9.6 MeV/nucleon). The mean charge fractions can be fitted to universal curves for both solid and gaseous strippers. Measurements of the equilibrium fraction of krypton ions at 1.04 MeV/nucleon passing through heavy vapours have shown that a higher average charge state is obtained than for lighter gaseous strippers. (Auth.)

Photoluminescence and reflectivity studies of high energy light ions irradiated polymethyl methacrylate films

Science.gov (United States)

Bharti, Madhu Lata; Singh, Fouran; Ramola, R. C.; Joshi, Veena

2017-11-01

The self-standing films of non-conducting polymethyl methacrylate (PMMA) were irradiated in vacuum using high energy light ions (HELIs) of 50 MeV Lithium (Li+3) and 80 MeV Carbon (C+5) at various ion dose to induce the optical changes in the films. Upon HELI irradiation, films exhibit a significant enhancement in optical reflectivity at the highest dose. Interestingly, the photoluminescence (PL) emission band with green light at (514.5 nm) shows a noticeable increase in the intensity with increasing ion dose for both ions. However, the rate of increase in PL intensity is different for both HELI and can be correlated with the linear energy transfer by these ions in the films. Origin of PL is attributed to the formation of carbon cluster and hydrogenated amorphous carbon in the polymer films. HAC clusters act as PL active centres with optical reflectivity. Most of the harmful radiation like UV are absorbed by the material and is becoming opaque after irradiation and this PL active material are useful in fabrication of optoelectronic devices, UV-filter, back-lit components in liquid crystal display systems, micro-components for integrate optical circuits, diffractive elements, advanced materials and are also applicable to the post irradiation laser treatment by means of ion irradiation.

Energy dispersive x-ray fluorescence spectrometric determination of phosphorus, calcium, iron, zinc, and strontium in human bones

International Nuclear Information System (INIS)

Ohta, Akishige; Matsubayashi, Takashi; Itoman, Moritoshi

1981-01-01

Phosphorus, calcium, iron, zinc and strontium in a human bone extracted by surgery were determined by energy dispersive X-ray fluorescence spectrometry. The bone was decomposed with nitric acid, then diluted with water. A specific quantity of the solution was naturally dried on polyethylene film, and subjected to X-ray analysis. For determining the calibration curves in a mixture of phosphorus, calcium, iron, zinc and strontium, for the analysis of phosphorus and calcium, germanium was used as the secondary target and aluminum as the filter; and for the analysis of iron, zinc and strontium, molybdenum and molybdenum-aluminum were used, respectively. Consequently, the calibration curves were able to be obtained with high precision in the ranges from 5 to 500 μg of phosphorus, from 1 to 50 μg of calcium and from 0.1 to 1.0 μg of iron, zinc and strontium. In this way, in 1 mg of the human bone by wet weight, phosphorus, calcium, iron, zinc and strontium were able to be determined. (J.P.N.)

Interaction of low-energy highly charged ions with matter; Wechselwirkung niederenergetischer hochgeladener Ionen mit Materie

Energy Technology Data Exchange (ETDEWEB)

Ginzel, Rainer

2010-06-09

The thesis presented herein deals with experimental studies of the interaction between highly charged ions and neutral matter at low collision energies. The energy range investigated is of great interest for the understanding of both charge exchange reactions between ions comprising the solar wind and various astrophysical gases, as well as the creation of near-surface nanostructures. Over the course of this thesis an experimental setup was constructed, capable of reducing the kinetic energy of incoming ions by two orders of magnitude and finally focussing the decelerated ion beam onto a solid or gaseous target. A coincidence method was employed for the simultaneous detection of photons emitted during the charge exchange process together with the corresponding projectile ions. In this manner, it was possible to separate reaction channels, whose superposition presumably propagated large uncertainties and systematic errors in previous measurements. This work has unveiled unexpectedly strong contributions of slow radiative decay channels and clear evidence of previously only postulated decay processes in charge exchange-induced X-ray spectra. (orig.)

Review of high excitation energy structures in heavy ion collisions: target excitations and three body processes

International Nuclear Information System (INIS)

Frascaria, N.

1987-09-01

A review of experimental results on high excitation energy structures in heavy ion inelastic scattering is presented. The contribution to the spectra of the pick-up break-up mechanism is discussed in the light of the data obtained with light heavy ion projectiles. Recent results obtained with 40 Ar beams at various energies will show that target excitations contribute strongly to the measured cross section

Rechargeable Lithium-Ion Based Batteries and Thermal Management for Airborne High Energy Electric Lasers (Preprint)

National Research Council Canada - National Science Library

Fellner, Joseph P; Miller, Ryan M; Shanmugasundaram, Venkatrama

2006-01-01

...). Rechargeable lithium-ion polymer batteries, for applications such as remote-control aircraft, are achieving simultaneously high energy density and high power density (>160 Whr/kg at > 1.0 kW/kg...

Mean excitation energies for molecular ions

Energy Technology Data Exchange (ETDEWEB)

Jensen, Phillip W.K.; Sauer, Stephan P.A. [Department of Chemistry, University of Copenhagen, Copenhagen (Denmark); Oddershede, Jens [Department of Physics, Chemistry, and Pharmacy, University of Southern Denmark, Odense (Denmark); Quantum Theory Project, Departments of Physics and Chemistry, University of Florida, Gainesville, FL (United States); Sabin, John R., E-mail: sabin@qtp.ufl.edu [Department of Physics, Chemistry, and Pharmacy, University of Southern Denmark, Odense (Denmark); Quantum Theory Project, Departments of Physics and Chemistry, University of Florida, Gainesville, FL (United States)

2017-03-01

The essential material constant that determines the bulk of the stopping power of high energy projectiles, the mean excitation energy, is calculated for a range of smaller molecular ions using the RPA method. It is demonstrated that the mean excitation energy of both molecules and atoms increase with ionic charge. However, while the mean excitation energies of atoms also increase with atomic number, the opposite is the case for mean excitation energies for molecules and molecular ions. The origin of these effects is explained by considering the spectral representation of the excited state contributing to the mean excitation energy.

Quantitative evaluation of high-energy O− ion particle flux in a DC magnetron sputter plasma with an indium-tin-oxide target

International Nuclear Information System (INIS)

Suyama, Taku; Bae, Hansin; Setaka, Kenta; Ogawa, Hayato; Fukuoka, Yushi; Suzuki, Haruka; Toyoda, Hirotaka

2017-01-01

O − ion flux from the indium tin oxide (ITO) sputter target under Ar ion bombardment is quantitatively evaluated using a calorimetry method. Using a mass spectrometer with an energy analyzer, O − energy distribution is measured with spatial dependence. Directional high-energy O − ion ejected from the target surface is observed. Using a calorimetry method, localized heat flux originated from high-energy O − ion is measured. From absolute evaluation of the heat flux from O − ion, O − particle flux in order of 10 18 m −2 s −1 is evaluated at a distance of 10 cm from the target. Production yield of O − ion on the ITO target by one Ar + ion impingement at a kinetic energy of 244 eV is estimated to be 3.3  ×  10 −3 as the minimum value. (paper)

Low energy ion beam dynamics of NANOGAN ECR ion source

Energy Technology Data Exchange (ETDEWEB)

Kumar, Sarvesh, E-mail: sarvesh@iuac.res.in; Mandal, A.

2016-04-01

A new low energy ion beam facility (LEIBF) has been developed for providing the mass analyzed highly charged intense ion beams of energy ranging from a few tens of keV to a few MeV for atomic, molecular and materials sciences research. The new facility consists of an all permanent magnet 10 GHz electron cyclotron resonance (ECR) ion source (NANOGAN) installed on a high voltage platform (400 kV) which provides large currents of multiply charged ion beams. Higher emittance at low energy of intense ion beam puts a tremendous challenge to the beam optical design of this facility. The beam line consists of mainly the electrostatic quadrupoles, an accelerating section, analyzing cum switching magnet and suitable beam diagnostics including vacuum components. The accelerated ion beam is analyzed for a particular mass to charge (m/q) ratio as well as guided to three different lines along 75°, 90° and 105° using a large acceptance analyzing cum switching magnet. The details of transverse beam optics to all the beam lines with TRANSPORT and GICOSY beam optics codes are being described. Field computation code, OPERA 3D has been utilized to design the magnets and electrostatic quadrupoles. A theoretical estimation of emittance for optimized geometry of ion source is given so as to form the basis of beam optics calculations. The method of quadrupole scan of the beam is used to characterize the emittance of the final beam on the target. The measured beam emittance increases with m/q ratios of various ion beams similar to the trend observed theoretically.

Development of the negative ion source at the National Laboratory for High Energy Physics

Energy Technology Data Exchange (ETDEWEB)

Takagi, Akira [National Lab. for High Energy Physics, Tsukuba, Ibaraki (Japan)

1997-02-01

On formation of direct high frequency chopped negative hydrogen ion beam from surface forming type negative hydrogen ion source, incident acceleration due to proton synchrotron was tried for a forming experiment and its application. By overlapping a high frequency pulse onto a bias DC voltage of convertor electrode, control of formation of negative hydrogen ion with high speed RF pulse of 2 MHz could be realized. And, incidence into 12 GeV proton accelerator to catch RF particles with waiting bucket system due to booster synchrotron, was effective for control of longitudinal emittance in the booster synchrotron. As a result, controls of the beam width and shape emitted from the booster synchrotron were possible. On application of high speed chopped negative hydrogen ion beam to accelerator, improvement of beam capture efficiency to the accelerated RF bucket, control of longitudinal emittance of accelerated beam, beam measurement at incidence into the accelerator and so forth were conducted. In this paper, results of the high speed chopped beam formation experiment using surface plasma forming type negative ion source and application of high speed beam chopping method synchronized with high frequency pulse at the National Laboratory of High Energy Physics are described. (G.K.)

Electron capture by highly charged low-velocity ions

International Nuclear Information System (INIS)

Cocke, C.L.; Dubois, R.; Justiniano, E.; Gray, T.J.; Can, C.

1982-01-01

This paper describes the use of a fast heavy ion beam to produce, by bombardment of gaseous targets, highly-charged low-velocity recoil ions, and the use of these secondary ions in turn as projectiles in studies of electron capture and ionization in low-energy collision systems. The interest in collisions involving low-energy highly-charged projectiles comes both from the somewhat simplifying aspects of the physics which attend the long-range capture and from applications to fusion plasmas, astrophysics and more speculative technology such as the production of X-ray lasers. The ions of interest in such applications should have both electronic excitation and center-of-mass energies in the keV range and cannot be produced by simply stripping fast heavy ion beams. Several novel types of ion source have been developed to produce low-energy highly-charged ions, of which the secondary ion recoil source discussed in this paper is one. (Auth.)

Black phosphorus induced photo-doping for high-performance organic-silicon heterojunction photovoltaics

Institute of Scientific and Technical Information of China (English)

Zhouhui Xia; Pengfei Li; Yuqiang Liu; Tao Song; Qiaoliang Bao; Shuit-Tong Lee; Baoquan Sun

2017-01-01

In conventional crystalline silicon (Si) homojunction solar cells,a strategy of doping by transporting phosphorus or boron impurities into Si is commonly used to build Ohmic contacts at rear electrodes.However,this technique involves an energy intensive,high temperature (～ 800 ℃) process and toxic doping materials.Black phosphorus (BP) is a two-dimensional,narrow bandgap semiconductor with high carrier mobility that exhibits broad light harvesting properties.Here,we place BP:zinc oxide (ZnO) composite films between Si and aluminum (Al) to improve their contact.Once the BP harvests photons with energies below 1.1 eV from the crystalline Si,the ZnO carrier concentration increases dramatically due to charge injection.This photo-induced doping results in a high carrier concentration in the ZnO film,mimicking the modulated doping technique used in semiconductor heterojunctions.We show that photo-induced carriers dramatically increase the conductivities of the BP-modified ZnO films,thus reducing the contact resistance between Si and Al.A photovoltaic power conversion efficiency of 15.2％ is achieved in organic-Si heterojunction solar cells that use a ZnO:BP layer.These findings demonstrate an effective way of improving Si/metal contact via a simple,low temperature process.

Surface modifications of polypropylene by high energy carbon ions

International Nuclear Information System (INIS)

Saha, A.; Chakraborty, V.; Dutta, R.K.; Chintalapudi, S.N.

2000-01-01

Polypropylene was irradiated with 12 C ions of 3.6 and 5.4 MeV energies using 3 MV tandem accelerator. The surface modification was investigated by Scanning Electron Microscopy (SEM). Optical changes were monitored by UV-VIS and FTIR spectroscopy. At the lowest ion fluence, only blister formation of various sizes (1-6 μm) was observed. Polymer when irradiated at a fluence of 1x10 14 ions/cm 2 exhibited a network structure. A comparative study on dose dependence of surface and bulk modification has been described. (author)

Energy dissipation of highly charged ions interacting with solid surfaces; Energieeintrag langsamer hochgeladener Ionen in Festkoerperoberflaechen

Energy Technology Data Exchange (ETDEWEB)

Kost, D.

2006-07-01

Motivated by the incomplete scientific description of the relaxation of highly charged ions in front of solid surfaces and their energy balance, this thesis describes an advanced complementary study of determining deposited fractions and re-emitted fractions of the potential energy of highly charged ions. On one side, a calorimetric measurement setup is used to determine the retained potential energy and on the other side, energy resolved electron spectroscopy is used for measuring the reemitted energy due to secondary electron emission. In order to study the mechanism of energy retention in detail, materials with different electronic structures are investigated: Cu, n-Si, p-Si and SiO{sub 2}. In the case of calorimetry, a linear relationship between the deposited potential energy and the inner potential energy of the ions was determined. The total potential energy which stays in the solid remains almost constant at about (80 {+-} 10) %. Comparing the results of the Cu, n-Si and p-Si targets, no significant difference could be shown. Therefore we conclude that the difference in energy deposition between copper, n-doped Si and p-doped Si is below 10 %, which is significantly lower than using SiO{sub 2} targets. For this purpose, electron spectroscopy provides a complementary result. For Cu and Si surfaces, an almost linear increase of the re-emitted energy with increasing potential energy of the ion up to Ar{sup 7+} was also observed. The ratio of the re-emitted energy is about (10 {+-} 5) % of the total potential energy of the incoming ion, almost independent of the ion charge state. In contrast, an almost vanishing electron emission was observed for SiO{sub 2} and for charge states below q=7. For Ar{sup 8+} and Ar{sup 9+}, the electron emission increased due to the contribution of the projectile LMM Auger electrons and the re-emitted energy amounts up to 20 % for Cu and Si and around 10 % for SiO{sub 2}. These results are in good agreement with the calorimetric

Enhancement of lipid accumulation by oleaginous yeast through phosphorus limitation under high content of ammonia.

Science.gov (United States)

Huang, Xiangfeng; Luo, Huijuan; Mu, Tianshuai; Shen, Yi; Yuan, Ming; Liu, Jia

2018-04-18

Low concentrations of acetic acid were used as carbon source to cultivate Cryptococcus curvatus MUCL 29819 for lipid production under high content of ammonia. Phosphorus limitation combined with initial pH regulation (pH = 6) weakened inhibition of free ammonia and promoted lipid accumulation. In batch cultivation, the produced lipid content and yield was 30.3% and 0.92 g/L, higher than those under unlimited condition (18.3% and 0.64 g/L). The content of monounsaturated fatty acid also increased from 37.3% (unlimited condition) to 45.8% (phosphorus-limited condition). During sequencing batch cultivation (SBC), the lipid content reached up to 51.02% under phosphorus-limited condition while only 31.88% under unlimited condition, which can be explained by the higher conversion efficiency of the carbon source to lipid. The total energy consumption including lipid extraction, transesterification and purification was 7.47 and 8.33 GJ under phosphorus-limited and unlimited condition, respectively. Copyright © 2018. Published by Elsevier Ltd.

Magnetic fusion with high energy self-colliding ion beams

International Nuclear Information System (INIS)

Restoker, N.; Wessel, F.; Maglich, B.; Fisher, A.

1993-01-01

Field-reversed configurations of energetic large orbit ions with neutralizing electrons have been proposed as the basis of a fusion reactor. Vlasov equilibria consisting of a ring or an annulus have been investigated. A stability analysis has been carried out for a long thin layer of energetic ions in a low density background plasma. There is a growing body of experimental evidence from tokamaks that energetic ions slow down and diffuse in accordance with classical theory in the presence of large non-thermal fluctuations and anomalous transport of low energy (10 keV) ions. Provided that major instabilities are under control, it seems likely that the design of a reactor featuring energetic self-colliding ion beams can be based on classical theory. In this case a confinement system that is much better than a tokamak is possible. Several methods are described for creating field reversed configurations with intense neutralized ion beams

Magnetic fusion with high energy self-colliding ion beams

International Nuclear Information System (INIS)

Rostoker, N.; Wessel, F.; Maglich, B.; Fisher, A.

1992-06-01

Field-reversed configurations of energetic large orbit ions with neutralizing electrons have been proposed as the basis of a fusion reactor. Vlasov equilibria consisting of a ring or an annulus have been investigated. A stability analysis has been carried out for a long thin layer of energetic ions in a low density background plasma. There is a growing body of experimental evidence from tokamaks that energetic ions slow down and diffuse in accordance with classical theory in the presence of large non-thermal fluctuations and anomalous transport of low energy (10 keV) ions. Provided that major instabilities are under control, it seems likely that the design of a reactor featuring energetic self-colliding ion beams can be based on classical theory. In this case a confinement system that is much better than a tokamak is possible. Several methods are described for creating field reversed configurations with intense neutralized ion beams

Production of High-Intensity, Highly Charged Ions

CERN Document Server

Gammino, S.

2013-12-16

In the past three decades, the development of nuclear physics facilities for fundamental and applied science purposes has required an increasing current of multicharged ion beams. Multiple ionization implies the formation of dense and energetic plasmas, which, in turn, requires specific plasma trapping configurations. Two types of ion source have been able to produce very high charge states in a reliable and reproducible way: electron beam ion sources (EBIS) and electron cyclotron resonance ion sources (ECRIS). Multiple ionization is also obtained in laser-generated plasmas (laser ion sources (LIS)), where the high-energy electrons and the extremely high electron density allow step-by-step ionization, but the reproducibility is poor. This chapter discusses the atomic physics background at the basis of the production of highly charged ions and describes the scientific and technological features of the most advanced ion sources. Particular attention is paid to ECRIS and the latest developments, since they now r...

Measurement of Anomalously Strong Emission from the 1s-9p Transition in the Spectrum of H-like Phosphorus Following Charge Exchange with Molecular Hydrogen

Science.gov (United States)

Leutenegger, M. A.; Beiersdorfer, P.; Brown, G. V.; Kelley, R. L.; Porter, F. S.

2010-01-01

We have measured K-shell x-ray spectra of highly ionized argon and phosphorus following charge exchange with molecular hydrogen at low collision energy in an electron beam ion trap using an x-ray calorimeter array with approx.6 eV resolution. We find that the emission at the high-end of the Lyman series is greater by a factor of two for phosphorus than for argon, even though the measurement was performed concurrently and the atomic numbers are similar. This does not agree with current theoretical models and deviates from the trend observed in previous measurements.

Multi-step intramolecular excitation energy transfer in dendritic pyrene-phosphorus(V)porphyrin heptads

Energy Technology Data Exchange (ETDEWEB)

Hirakawa, Kazutaka, E-mail: hirakawa.kazutaka@shizuoka.ac.jp [Applied Chemistry and Biochemical Engineering Course, Department of Engineering, Graduate School of Integrated Science and Technology, Shizuoka University, Johoku 3-5-1, Naka-ku, Hamamatsu, Shizuoka 432-8561 (Japan); Department of Optoelectronics and Nanostructure Science, Graduate School of Science and Technology, Shizuoka University, Johoku 3-5-1, Naka-ku, Hamamatsu, Shizuoka 432-8561 (Japan); Segawa, Hiroshi [Department of Multi-Disciplinary Science - General Systems Studies, Graduate School of Arts and Sciences, The University of Tokyo, Komaba 3-8-1, Meguro-ku, Tokyo 153-8904 (Japan); Research Center for Advanced Science and Technology, The University of Tokyo, Komaba 4-6-1, Meguro-ku, Tokyo 153-8904 (Japan)

2016-11-15

Dendritic heptad molecules in which four pyrenyl groups are connected at the central phosphorus atom of the edge-porphyrins of the center-to-edge type porphyrin trimers were synthesized to investigate a multi-step excitation energy transfer. As the central energy acceptor, two types porphyrins which one was phosphorus(V)tetraphenylporphyrin (H2) and another was its derivative substituted by butoxy groups at four para-position of meso-phenyl groups (H1) were used. In the photoexcited state of the pyrene units, the excitation energy transfer to the central-porphyrin unit was observed in toluene. The excitation energy transfer is considered to be through two pathways; one is a stepwise pathway through the edge-porphyrin unit and another is a direct excitation energy transfer to the central porphyrin. The direct excitation energy transfer from pyrenes to the edge-porphyrin and central-porphyrin were observed in the case for H1. From the excited state of the edge-porphyrins, the excitation energy transfer to the central-porphyrin occurs in the H1 case. In the H2 case, the excitation energy of central-porphyrin is higher than that of H1, and the electron transfer from edge-porphyrin to the central-porphyrin become predominant process. - Highlights: • Dendritic pyrene-porphyrin heptads were synthesized. • Excitation energy transfer occurs from the pyrenyl moiety to the phosphorus(V)porphyrin. • The stepwise and direct energy transfer pathways were observed. • The quantum yields of these energy transfer pathways could be determined.

Multi-step intramolecular excitation energy transfer in dendritic pyrene-phosphorus(V)porphyrin heptads

International Nuclear Information System (INIS)

Hirakawa, Kazutaka; Segawa, Hiroshi

2016-01-01

Dendritic heptad molecules in which four pyrenyl groups are connected at the central phosphorus atom of the edge-porphyrins of the center-to-edge type porphyrin trimers were synthesized to investigate a multi-step excitation energy transfer. As the central energy acceptor, two types porphyrins which one was phosphorus(V)tetraphenylporphyrin (H2) and another was its derivative substituted by butoxy groups at four para-position of meso-phenyl groups (H1) were used. In the photoexcited state of the pyrene units, the excitation energy transfer to the central-porphyrin unit was observed in toluene. The excitation energy transfer is considered to be through two pathways; one is a stepwise pathway through the edge-porphyrin unit and another is a direct excitation energy transfer to the central porphyrin. The direct excitation energy transfer from pyrenes to the edge-porphyrin and central-porphyrin were observed in the case for H1. From the excited state of the edge-porphyrins, the excitation energy transfer to the central-porphyrin occurs in the H1 case. In the H2 case, the excitation energy of central-porphyrin is higher than that of H1, and the electron transfer from edge-porphyrin to the central-porphyrin become predominant process. - Highlights: • Dendritic pyrene-porphyrin heptads were synthesized. • Excitation energy transfer occurs from the pyrenyl moiety to the phosphorus(V)porphyrin. • The stepwise and direct energy transfer pathways were observed. • The quantum yields of these energy transfer pathways could be determined.

SIS: an accelerator installation for heavy ions of high energy

International Nuclear Information System (INIS)

The two major sections of the report cover the scientific experimental program and the accelerator installation. Topics covered in the first include: heavy ion physics in the medium energy region; nuclear physics at relativistic energies; atomic physics loss and capture cross sections for electrons; spectroscopy of few-electron systems; atomic collision processes; biological experiments; nuclear track techniques in biology; and experiments with protons and secondary radiation. The second includes: concept for the total installation; technical description of the SIS 12; technical description of the SIS 100; status of the UNILAC injector; development options for the SIS installations; properties of the heavy ion beam; and structural work and technical supply provisions. In this SIS project proposal, an accelerator installation based on two synchrotrons is described with which atomic nuclei up to uranium can be accelerated to energies of more than 10 GeV/μ. With the SIS 12, which is the name of the first stage, heavy ion physics at intermediate energies can be pursued up to 500 MeV/μ. The second stage, a larger synchrotron, the SIS 100, has a diameter of 250 m. With this device, it is proposed to open up the domain of relativistic heavy ion physics up to 14 GeV/μ (for intermediate mass particles) and 10 GeV/μ (for uranium)

Bevalac, a high-energy heavy-ion facility: status and outlook

International Nuclear Information System (INIS)

Grunder, H.A.

1974-01-01

The high-energy heavy-ion facility, which has commonly been referred to as the Bevalac, is a synchrotron with B rho of 9000 [kG-in or 2.3 x 10 2 kG-m] having special injectors. The synchrotron has three injectors. The 50 MeV proton injector, originally from BNL, is a tool left over from the high-energy high-intensity days of this productive synchrotron. The 20 MeV linac is a proton linac, designed so conservatively that it was possible to accelerate modest but useful beams of 12 C, 14 N, and 16 O as well as deuterons and alpha particles in the 2 β lambda mode. This was accomplished in 1971. After our first trials, a suggestion made earlier by A. Ghiorso to inject from the SuperHILAC into the synchrotron was actively pursued. Reasons as to why the SuperHILAC is being used as injector to the Bevatron are given

Chemical and structural effects of phosphorus on the corrosion behavior of ion beam mixed Fe-Cr-P alloys

International Nuclear Information System (INIS)

Demaree, J.D.; Was, G.S.; Sorensen, N.R.

1992-01-01

An experimental program was conducted to determine the mechanisms by which phosphorus affects the corrosion and passivation behavior of Fe-Cr-P alloys. To identify separately the effects of structure and chemistry on the corrosion behavior, thin films of Fe-10Cr-xP (0≤x≤35 at.%) were prepared by ion beam mixing. Films with a phosphorus content greater than approximately 20at.% were found to be entirely amorphous. Devitrification of the amorphous phase was accomplished by heating the samples to 450degC in an inert environment. Standard polarization tests of the sulfuric acid (with and without Cl - ) indicated that the films containing phosphorus were more corrosion resistant than Fe-10Cr, at both active and passive potentials. There was a monotonic relationship between the amount of phosphorus in the alloy and the corrosion resistance, with the open-circuit corrosion rate of Fe-10Cr-35P nearly four orders of magnitude lower than that of Fe-10Cr. Devitrification of the alloys had no significant effect on the corrosion rate, indicating that the primary effect of phosphorus is chemical in nature, and not structural. The passive oxides were depth-profiled using X-ray photoelectron spectroscopy, which indicated that phosphorus was a primary constituent, as phosphate. The presence of phosphate in the passive oxides reduced the overall corrosion rate directly, by suppressing anodic dissolution. The presence of phosphorus did enhance chromium enrichment in the oxide, but that was not thought to be the primary mechanism by which phosphorus increased the corrosion resistance. (orig.)

Experimental heavy ion physics at high energies. Progress report, September 1992--November 1993

Energy Technology Data Exchange (ETDEWEB)

1993-12-31

This report summarizes the research activities of the experimental high energy heavy ion physics group at Vanderbilt University carried out under Grant No. DE-FG05092ER40712 with the Department of Energy during the period Oct 1, 1992 to Nov 30, 1993. This research encompasses four areas of related inquiry in relativistic and high energy nuclear reactions. The preparation of the PHENIX experiment which has been approved as one of the two major experiments at RHIC to start in 1998. The RD10/RD45 Muon Identifier experiment which will provide essential input for the design of the Muon Endcap arm detector sub-system in PHENIX. The E855 Soft Photon Experiment at the AGS designed to clarify the status of a possible quark-gluon-plasma signature with presently available heavy-ion collisions. The construction CsI Ball detector project at Texas A&M which is designed as part of a comprehensive detector system which will probe the nuclear equation of state in the 50 MeV/nucleon domain.

An ion beam deceleration lens for ultra-low-energy ion bombardment of naked DNA

Energy Technology Data Exchange (ETDEWEB)

Thopan, P.; Prakrajang, K. [Plasma and Beam Physics Research Facility, Department of Physics and Materials Science, Faculty of Science, Chiang Mai University, Chiang Mai 50200 (Thailand); Thongkumkoon, P. [Plasma and Beam Physics Research Facility, Department of Physics and Materials Science, Faculty of Science, Chiang Mai University, Chiang Mai 50200 (Thailand); Thailand Center of Excellence in Physics, Commission on Higher Education, 328 Si Ayutthaya Road, Bangkok 10400 (Thailand); Suwannakachorn, D. [Plasma and Beam Physics Research Facility, Department of Physics and Materials Science, Faculty of Science, Chiang Mai University, Chiang Mai 50200 (Thailand); Yu, L.D., E-mail: yuldyuld@gmail.com [Plasma and Beam Physics Research Facility, Department of Physics and Materials Science, Faculty of Science, Chiang Mai University, Chiang Mai 50200 (Thailand); Thailand Center of Excellence in Physics, Commission on Higher Education, 328 Si Ayutthaya Road, Bangkok 10400 (Thailand)

2013-07-15

Highlights: ► An ion beam deceleration lens was designed and constructed. ► The deceleration lens was installed and tested. ► The decelerated ion beam energy was measured using an electrical field. ► Decelerated ultra-low-energy ion beam bombarded naked DNA. ► Ion beam with energy of a few tens of eV could break DNA strands. -- Abstract: Study of low-energy ion bombardment effect on biological living materials is of significance. High-energy ion beam irradiation of biological materials such as organs and cells has no doubt biological effects. However, ion energy deposition in the ion-bombarded materials dominantly occurs in the low-energy range. To investigate effects from very-low-energy ion bombardment on biological materials, an ion beam deceleration lens is necessary for uniform ion energy lower than keV. A deceleration lens was designed and constructed based on study of the beam optics using the SIMION program. The lens consisted of six electrodes, able to focus and decelerate primary ion beam, with the last one being a long tube to obtain a parallel uniform exiting beam. The deceleration lens was installed to our 30-kV bioengineering-specialized ion beam line. The final decelerated-ion energy was measured using a simple electrostatic field to bend the beam to range from 10 eV to 1 keV controlled by the lens parameters and the primary beam condition. In a preliminary test, nitrogen ion beam at 60 eV decelerated from a primary 20-keV beam bombarded naked plasmid DNA. The original DNA supercoiled form was found to change to relaxed and linear forms, indicating single or double strand breaks. The study demonstrated that the ion bombardment with energy as low as several-tens eV was possible to break DNA strands and thus potential to cause genetic modification of biological cells.

An ion beam deceleration lens for ultra-low-energy ion bombardment of naked DNA

International Nuclear Information System (INIS)

Thopan, P.; Prakrajang, K.; Thongkumkoon, P.; Suwannakachorn, D.; Yu, L.D.

2013-01-01

Highlights: ► An ion beam deceleration lens was designed and constructed. ► The deceleration lens was installed and tested. ► The decelerated ion beam energy was measured using an electrical field. ► Decelerated ultra-low-energy ion beam bombarded naked DNA. ► Ion beam with energy of a few tens of eV could break DNA strands. -- Abstract: Study of low-energy ion bombardment effect on biological living materials is of significance. High-energy ion beam irradiation of biological materials such as organs and cells has no doubt biological effects. However, ion energy deposition in the ion-bombarded materials dominantly occurs in the low-energy range. To investigate effects from very-low-energy ion bombardment on biological materials, an ion beam deceleration lens is necessary for uniform ion energy lower than keV. A deceleration lens was designed and constructed based on study of the beam optics using the SIMION program. The lens consisted of six electrodes, able to focus and decelerate primary ion beam, with the last one being a long tube to obtain a parallel uniform exiting beam. The deceleration lens was installed to our 30-kV bioengineering-specialized ion beam line. The final decelerated-ion energy was measured using a simple electrostatic field to bend the beam to range from 10 eV to 1 keV controlled by the lens parameters and the primary beam condition. In a preliminary test, nitrogen ion beam at 60 eV decelerated from a primary 20-keV beam bombarded naked plasmid DNA. The original DNA supercoiled form was found to change to relaxed and linear forms, indicating single or double strand breaks. The study demonstrated that the ion bombardment with energy as low as several-tens eV was possible to break DNA strands and thus potential to cause genetic modification of biological cells

Impacts of anthropic pressures on soil phosphorus availability, concentration, and phosphorus forms in sediments in a Southern Brazilian watershed

Energy Technology Data Exchange (ETDEWEB)

Pellegrini, Joao Batista Rossetto; Rheinheimer dos Santos, Danilo; Goncalves, Celso Santos; Copetti, Andre Carlos Cruz [Dept. de Solos, Univ. Federal de Santa Maria, Centro de Ciencias Rurais, Santa Maria, RS (Brazil); Bortoluzzi, Edson Campanhola [Faculdade de Agronomia e Medicina Veterinaria da Univ. de Passo Fundo, RS (Brazil); Tessier, Daniel [Inst. National de la Recherche Agronomique, Versailles (France)

2010-04-15

Purpose: The transfer of soil sediments and phosphorus from terrestrial to aquatic systems is a common process in agricultural lands. The aims of this paper are to quantify the soil phosphorus availability and to characterize phosphorus forms in soil sediments as contaminant agents of waters as a function of anthropic pressures. Materials and methods On three subwatersheds with different anthropic pressure, water and sediment samples were collected automatically in upstream and downstream discharge points in six rainfall events during the tobacco growing season. Phosphorus desorption capacity from soil sediments was estimated by successive extractions with anion exchange resins. First-order kinetic models were adjusted to desorption curves for estimating potentially bioavailable particulate phosphorus, desorption rate constant, and bioavailable particulate phosphorus. Results and discussion The amount of bioavailable particulate phosphorus was directly correlated with the iron oxide content. The value of desorption rate constant was directly related with the total organic carbon and inversely with the iron oxide contents. Phosphate ions were released to solution, on average, twice as rapidly from sediments collected in subwatersheds with low anthropic activity than from those ones of highly anthropic subwatersheds. Anthropic pressure on watershed can engender high sediment discharge, but these solid particles seem to present low phosphorus-releasing capacity to water during transport due to the evidenced high affinity between phosphorus and iron oxide from sediments. Conclusions Anthropic pressure was related with sediment concentration and phosphorus release to aquatic systems. While natural vegetation along streams plays a role on soil and water depuration, it is unable to eliminate the phosphorus inputs intrinsic to the agricultural-intensive systems. Recommendations and perspectives The contamination of water in watershed by phosphates is facilitated by the

Mechanical properties of low alloy high phosphorus weathering steel

Directory of Open Access Journals (Sweden)

Jena B.K.

2015-01-01

Full Text Available Mechanical behaviour of two low alloy steels (G11 and G12 was studied with respect to different phosphorus contents. Tensile strength and yield strength increased while percentage elongation at fracture decreased on increasing phosphorus content. The SEM and light optical photomicrograph of low phosphorus steel (G11 revealed ferrite and pearlite microstructure. On increasing phosphorus content from 0.25 wt.% to 0.42 wt.%, the morphology of grain changed from equiaxed shape to pan-cake shape and grain size also increased. The Charpy V notch (CVN impact energy of G11 and G12 steel at room temperature was 32 J and 4 J respectively and their fractographs revealed brittle rupture with cleavage facets for both the steels. However, the fractograph of G11 steel after tensile test exhibited ductile mode of fracture with conical equiaxed dimple while that of G12 steel containing 0.42 wt. % P exhibited transgranular cleavage fracture. Based on this study, G11 steel containing 0.25 wt. % P could be explored as a candidate material for weathering application purpose where the 20°C toughness requirement is 27 J as per CSN EN10025-2:2004 specification.

Preparation of phosphorus targets using the compound phosphorus nitride

International Nuclear Information System (INIS)

Maier-Komor, P.

1987-01-01

Commercially available phosphorus nitride (P 3 N 5 ) shows a high oxygen content. Nevertheless, this material is attractive for use as phosphorus targets in experiments where red phosphorus would disappear due to its high vapor pressure and where a metal partner in the phosphide must be excluded due to its high atomic number. Methods are described to produce phosphorus nitride targets by vacuum evaporation condensation. (orig.)

Low-energy ion outflow modulated by the solar wind energy input

Science.gov (United States)

Li, Kun; Wei, Yong; Andre, Mats; Eriksson, Anders; Haaland, Stein; Kronberg, Elena; Nilsson, Hans; Maes, Lukas

2017-04-01

Due to the spacecraft charging issue, it has been difficult to measure low-energy ions of ionospheric origin in the magnetosphere. A recent study taking advantage of the spacecraft electric potential has found that the previously 'hidden' low-energy ions is dominant in the magnetosphere. This comprehensive dataset of low-energy ions allows us to study the relationship between the ionospheric outflow and energy input from the solar wind (ɛ). In this study, we discuss the ratios of the solar wind energy input to the energy of the ionospheric outflow. We show that the ɛ controls the ionospheric outflow when the ɛ is high, while the ionospheric outflow does not systematically change with the ɛ when the ɛ is low.

Analysis of phosphorus herbicides by ion-pairing reversed-phase liquid chromatography coupled to inductively coupled plasma mass spectrometry with octapole reaction cell.

Science.gov (United States)

Sadi, Baki B M; Vonderheide, Anne P; Caruso, Joseph A

2004-09-24

A reversed phase ion-pairing high performance liquid chromatographic (RPIP-HPLC) method is developed for the separation of two phosphorus herbicides, Glufosinate and Glyphosate as well as Aminomethylphosphonic acid (AMPA), the major metabolite of Glyphosate. Tetrabutylammonium hydroxide is used as the ion-pairing reagent in conjunction with an ammonium acetate/acetic acid buffering system at pH 4.7. An inductively coupled plasma mass spectrometer (ICP-MS) is coupled to the chromatographic system to detect the herbicides at m/z = 31P. Historically, phosphorus has been recognized as one of the elements difficult to analyze in argon plasma. This is due to its relatively high ionization potential (10.5 eV) as well as the inherent presence of the polyatomic interferences 14N16O1H+ and 15N16O+ overlapping its only isotope at m/z = 31. An octapole reaction cell is utilized to minimize the isobaric polyatomic interferences and to obtain the highest signal-to-background ratio. Detection limits were found to be in the low ppt range (25-32 ng/l). The developed method is successfully applied to the analysis of water samples collected from the Ohio River and spiked with a standard compounds at a level of 20 microg/l.

Development of nano-structure controlled polymer electrolyte fuel-cell membranes by high-energy heavy ion irradiation

International Nuclear Information System (INIS)

Yamaki, Tetsuya; Asano, Masaharu; Maekawa, Yasunari; Yoshida, Masaru; Kobayashi, Misaki; Nomura, Kumiko; Takagi, Shigeharu

2008-01-01

There is increasing interest in polymer electrolyte fuel cells (PEFCs) together with recent worldwide energy demand and environmental issues. In order to develop proton-conductive membranes for PEFCs, we have been using high-energy heavy ion beams from the cyclotron accelerator of Takasaki Ion Accelerators for Advanced Radiation Application (TIARA), JAEA. Our strategic focus is centered on using nano-scale controllability of the ion-beam processing; the membrane preparation involves (1) the irradiation of commercially-available base polymer films with MeV ions, (2) graft polymerization of vinyl monomers into electronically-excited parts along the ion trajectory, called latent tracks, and (3) sulfonation of the graft polymers. Interestingly, the resulting membranes exhibited anisotropic proton transport, i.e., higher conductivity in the thickness direction. According to microscopic observations, this is probably because the columnar electrolyte phase extended, with a width of tens-to-hundreds nanometers, through the membrane. Other excellent membrane properties, e.g., sufficient mechanical strength, high dimensional stability, and low gas permeability should be due to such a controlled structure. (author)

High energy density in matter produced by heavy ion beams. Annual report 1987

International Nuclear Information System (INIS)

1988-08-01

Research activities presented in this annual report were carried out in 1987 in the framework of the government-funded program 'High Energy Density in Matter Produced by Heavy Ion Beams'. It addresses fundamental problems of the generation and investigation of hot dense matter. Its initial motivation and its ultimate goal is the question whether inertial confinement can be achieved by intense heavy ion beams. The new accelerator facility SIS/ESR now under construction at GSI will provide an excellent potential for research in this field. The construction work at the new validity is on schedule. The building construction is near completion and the SIS accelerator will have its first beam at the beginning of next year. First experiments at lower intensity will start in summer 1989 and the full program will run after the cooler and storage ring ESR has got operational. Accordingly, the planning and the preparation of the high energy density experiments at this unique facility was an essential part of the activities last year. In this funding period emphasis was given to the experimental activities at the existing accelerator. In addition to a number of accelerator-oriented and instrumental developments, an experiment on beam-plasma interaction had first exciting results, a significant increase of the stopping power for heavy ions in plasma was measured. Other important activities were the investigation of dielectronic recombination of highly charged ions, spectroscopic investigations aiming at the pumping of short wavelength lasers by heavy ion beams and a crossed beam experiment for the determination of Bi + + Bi + ionization cross sections. As in previous years theoretical work an space-charge dominated beam dynamics as well as on hydrodynamics of dense plasmas, radiation transport and beam plasma interaction was continued, thus providing a basis for the future experiments. (orig.)

Influence of high-energy ion implantation on the microstructure of Sn - 9,8 wt. % Zn alloy

International Nuclear Information System (INIS)

Gusakova, O.V.

2016-01-01

The results of investigation of influence of Xe ion implantation on the microstructure of Sn - 9,8 wt. % Zn alloy are represented/ Analysis of the experimental results shows that the high-energy ion implantation of Xe causes a change in the particle size of zinc. (authors)

"Doping" pentacene with sp(2)-phosphorus atoms: towards high performance ambipolar semiconductors.

Science.gov (United States)

Long, Guankui; Yang, Xuan; Chen, Wangqiao; Zhang, Mingtao; Zhao, Yang; Chen, Yongsheng; Zhang, Qichun

2016-01-28

Recent research progress in black phosphorus sheets strongly encourages us to employ pentacene as a parent system to systematically investigate how the "doping" of sp(2)-phosphorus atoms onto the backbone of pentacene influences its optical and charge transport properties. Our theoretical investigations proved that increasing the contribution of the pz atomic orbital of the sp(2)-phosphorus to the frontier molecular orbital of phosphapentacenes could significantly decrease both hole and electron reorganization energies and dramatically red-shift the absorption of pentacene. The record smallest hole and electron reorganization energies of 69.80 and 95.74 meV for heteropentacene derivatives were obtained. These results suggest that phosphapentacenes (or phosphaacenes) could be potential promising candidates to achieve both higher and balanced mobilities in organic field effect transistors and realize a better power conversion efficiency in organic photovoltaics.

Damage of copper by low energy xenon ions

International Nuclear Information System (INIS)

Babad-Zakhryapin, A.A.; Popenko, V.A.

1988-01-01

Changes in the copper crystal structure bombarded by xenon ions with 30-150 eV energy are studied. Foils of MOb copper mark, 10 mm in diameter and 100 μm thickness, are irradiated. The initial specimens are annealed in vacuum during 1 h at 900 K temperature. The specimens are bombarded by xenon ions in a water-cooled holder. A TE-O type accelerator serves as a xenon ion source. The ion energy varies within 30 to 150 eV range. The ion flux density is 8x10 16 ion/(cm 2 xs). It is shown that crystal structure variations at deep depths are observed not only at high (>1 keV), but at low ion energies down to several dozens of electronvolt as well. The crystal structure variation on copper irradiation by xenon ions with 30-150 eV energy is followed by formation of defects like dislocation loops, point defects in the irradiated target bulk

Carbon supported ultrafine gold phosphorus nanoparticles as highly efficient electrocatalyst for alkaline ethanol oxidation reaction

International Nuclear Information System (INIS)

Li, Tongfei; Fu, Gengtao; Su, Jiahui; Wang, Yi; Lv, Yinjie; Zou, Xiuyong; Zhu, Xiaoshu; Xu, Lin; Sun, Dongmei; Tang, Yawen

2017-01-01

Graphical abstract: We develop a new kind of carbon supported gold-phosphorus (Au-P/C) electrocatalyst by a facile and novel phosphorus reduction method, and demonstrate the Au-P/C is a highly active and stable electrocatalyst for the ethanol oxidation reaction. - Highlights: • Au-P/C catalyst is synthesized by a facile and novel white-phosphorus reduce method. • AuP particles with ultrafine particle-size are uniformly dispersed on carbon support. • Au-P/C catalyst exhibits much higher content of P 0 than reported metal/P catalysts. • Au-P/C catalysts show excellent catalytic properties for ethanol oxidation reaction. - Abstract: Herein, we develop a new kind of carbon supported gold-phosphorus (Au-P/C) electrocatalyst for the alkaline ethanol oxidation reaction (EOR). The Au-P/C catalysts with different Au/P ratio (i.e., AuP/C, Au 3 P 2 /C and Au 4 P 3 /C) can be obtained by a facile and novel hot-reflux method with white phosphorus (P 4 ) as reductant and ethanol as solvent. The crystal structure, composition and particle-size of the Au-P/C catalysts are investigated by X-ray diffraction (XRD), Energy Dispersive Spectrometer (EDS), scanning electron microscopy (SEM) and X-ray photoelectron spectroscopy (XPS), etc. The results demonstrate that Au-P/C catalysts present an alloy phase with the high content of P, ultrafine particle-size and high dispersity on carbon support, which results in excellent electrocatalytic activity and stability towards the EOR compared with that of the free-phosphorus Au/C catalyst. In addition, among the various Au-P/C catalysts with different Au/P ratio, the AuP/C sample exhibits the best electrocatalytic performance in comparison with other Au 3 P 2 /C and Au 4 P 3 /C samples.

Rapid determination of trace phosphorus, sulfur, chlorine, bromine and iodine by energy dispersive X-ray fluorescence analysis with monochromatic excitations

International Nuclear Information System (INIS)

Wakisaka, Tatsushi; Morita, Naoki; Hirabayashi, Tadashi; Nakahara, Taketoshi

1998-01-01

A useful and rapid procedure is described for the determination of trace phosphorus, sulfur, chlorine, bromine, and iodine by means of an energy dispersive X-ray fluorescence spectrometer (EDXRF) with monochromatic excitations. Using monochromatic excitations, the detection limits for phosphorus, sulfur, chlorine (Cr-Kα, 5.41 keV), bromine (Mo-Kα, 17.44 keV), and iodine (W-continuum, 40 keV) were found to be 4.6, 1.7, 0.7, 0.09 and 0.5 μg g -1 , respectively. The relative standard deviations in five replicate measurements were 0.9-1.3%. The proposed method was applied to the direct determination of sulfur in the NIST Residual Fuel Oil, and others. The results obtained by the proposed method were in good agreement with the certified values. Bromine in a seawater sample, as well as iodine and bromine in a brine sample were determined by the proposed method. The obtained results were in good agreement with those obtained by ion chromatography. (author)

Measurement of ultra-low ion energy of decelerated ion beam using a deflecting electric field

Energy Technology Data Exchange (ETDEWEB)

Thopan, P.; Suwannakachorn, D.; Tippawan, U. [Plasma and Beam Physics Research Facility, Department of Physics and Materials Science, Faculty of Science, Chiang Mai University, Chiang Mai 50200 (Thailand); Yu, L.D., E-mail: yuld@thep-center.org [Plasma and Beam Physics Research Facility, Department of Physics and Materials Science, Faculty of Science, Chiang Mai University, Chiang Mai 50200 (Thailand); Thailand Center of Excellence in Physics, Commission on Higher Education, 328 Si Ayutthaya Road, Bangkok 10400 (Thailand)

2015-12-15

In investigation on ultra-low-energy ion bombardment effect on DNA, an ion beam deceleration lens was developed for high-quality ultra-low-energy ion beam. Measurement of the ion energy after deceleration was necessary to confirm the ion beam really decelerated as theoretically predicted. In contrast to conventional methods, this work used a simple deflecting electrostatic field after the deceleration lens to bend the ion beam. The beam bending distance depended on the ion energy and was described and simulated. A system for the measurement of the ion beam energy was constructed. It consisted of a pair of parallel electrode plates to generate the deflecting electrical field, a copper rod measurement piece to detect ion beam current, a vernier caliper to mark the beam position, a stepping motor to translate the measurement rod, and a webcam-camera to read the beam bending distance. The entire system was installed after the ion-beam deceleration lens inside the large chamber of the bioengineering vertical ion beam line. Moving the measurement rod across the decelerated ion beam enabled to obtain beam profiles, from which the beam bending distance could be known and the ion beam energy could be calculated. The measurement results were in good agreement with theoretical and simulated results.

Mean excitation energies for molecular ions

DEFF Research Database (Denmark)

Jensen, Phillip W.K.; Sauer, Stephan P.A.; Oddershede, Jens

2017-01-01

The essential material constant that determines the bulk of the stopping power of high energy projectiles, the mean excitation energy, is calculated for a range of smaller molecular ions using the RPA method. It is demonstrated that the mean excitation energy of both molecules and atoms increase...

Independent control of ion current and ion impact energy onto electrodes in dual frequency plasma devices

International Nuclear Information System (INIS)

Boyle, P C; Ellingboe, A R; Turner, M M

2004-01-01

Dual frequency capacitive discharges are designed to offer independent control of the flux and energy of ions impacting on an object immersed in a plasma. This is desirable in applications such as the processing of silicon wafers for microelectronics manufacturing. In such discharges, a low frequency component couples predominantly to the ions, while a high frequency component couples predominantly to electrons. Thus, the low frequency component controls the ion energy, while the high frequency component controls the plasma density. Clearly, this desired behaviour is not achieved for arbitrary configurations of the discharge, and in general one expects some unwanted coupling of ion flux and energy. In this paper we use computer simulations with the particle-in-cell method to show that the most important governing parameter is the ratio of the driving frequencies. If the ratio of the high and low frequencies is great enough, essentially independent control of the ion energy and flux is possible by manipulation of the high and low frequency power sources. Other operating parameters, such as pressure, discharge geometry, and absolute power, are of much less significance

Influence of dense plasma on the energy levels and transition properties in highly charged ions

Science.gov (United States)

Chen, Zhan-Bin; Hu, Hong-Wei; Ma, Kun; Liu, Xiao-Bin; Guo, Xue-Ling; Li, Shuang; Zhu, Bo-Hong; Huang, Lian; Wang, Kai

2018-03-01

The studies of the influence of plasma environments on the level structures and transition properties for highly charged ions are presented. For the relativistic treatment, we implemented the multiconfiguration Dirac-Fock method incorporating the ion sphere (IS) model potential, in which the plasma screening is taken into account as a modified interaction potential between the electron and the nucleus. For the nonrelativistic treatment, analytical solutions of the Schrödinger equation with two types of the IS screened potential are proposed. The Ritz variation method is used with hydrogenic wave function as a trial wave function that contains two unknown variational parameters. Bound energies are derived from an energy equation, and the variational parameters are obtained from the minimisation condition of the expectation value of the energy. Numerical results for hydrogen-like ions in dense plasmas are presented as examples. A detailed analysis of the influence of relativistic effects on the energy levels and transition properties is also reported. Our results are compared with available results in the literature showing a good quantitative agreement.

Strong-field physics using lasers and relativistic heavy ions at the high-energy storage ring HESR at FAIR

International Nuclear Information System (INIS)

Kuehl, T; Bagnoud, V; Stoehlker, T; Litvinov, Y; Winters, D F A; Zielbauer, B; Backe, H; Spielmann, Ch; Seres, J; Tünnermann, A; Neumayer, P; Aurand, B; Namba, S; Zhao, H Y

2014-01-01

The HESR high-energy ion storage ring at FAIR will provide unprecedented possibilities for strong-field physics using novel laser sources on relativistic heavy ions. An overview on the planning will be given.

Formation of hexagonal silicon carbide by high energy ion beam irradiation on Si (1 0 0) substrate

International Nuclear Information System (INIS)

Bhuyan, H; Favre, M; Valderrama, E; Avaria, G; Chuaqui, H; Mitchell, I; Wyndham, E; Saavedra, R; Paulraj, M

2007-01-01

We report the investigation of high energy ion beam irradiation on Si (1 0 0) substrates at room temperature using a low energy plasma focus (PF) device operating in methane gas. The unexposed and ion exposed substrates were characterized by x-ray diffraction, scanning electron microscopy (SEM), photothermal beam deflection, energy-dispersive x-ray analysis and atomic force microscopy (AFM) and the results are reported. The interaction of the pulsed PF ion beams, with characteristic energy in the 60-450 keV range, with the Si surface, results in the formation of a surface layer of hexagonal silicon carbide. The SEM and AFM analyses indicate clear step bunching on the silicon carbide surface with an average step height of 50 nm and a terrace width of 800 nm

90 deg.Neutron emission from high energy protons and lead ions on a thin lead target

CERN Document Server

Agosteo, S; Foglio-Para, A; Mitaroff, W A; Silari, Marco; Ulrici, L

2002-01-01

The neutron emission from a relatively thin lead target bombarded by beams of high energy protons/pions and lead ions was measured at CERN in one of the secondary beam lines of the Super Proton Synchrotron for radiation protection and shielding calculations. Measurements were performed with three different beams: sup 2 sup 0 sup 8 Pb sup 8 sup 2 sup + lead ions at 40 GeV/c per nucleon and 158 GeV/c per nucleon, and 40 GeV/c mixed protons/pions. The neutron yield and spectral fluence per incident ion on target were measured at 90 deg.with respect to beam direction. Monte-Carlo simulations with the FLUKA code were performed for the case of protons and pions and the results found in good agreement with the experimental data. A comparison between simulations and experiment for protons, pions and lead ions have shown that--for such high energy heavy ion beams--a reasonable estimate can be carried out by scaling the result of a Monte-Carlo calculation for protons by the projectile mass number to the power of 0.80-0...

Phosphorus doped graphene by inductively coupled plasma and triphenylphosphine treatments

Energy Technology Data Exchange (ETDEWEB)

Shin, Dong-Wook, E-mail: shindong37@skku.edu; Kim, Tae Sung; Yoo, Ji-Beom, E-mail: jbyoo@skku.edu

2016-10-15

Highlights: • Substitution doping is a promising method for opening the energy band gap of graphene. • Substitution doping with phosphorus in the graphene lattice has numerous advantage such as high band gap, low formation energy, and high net charge density compared to nitrogen. • V{sub dirac} of Inductively coupled plasma (ICP) and triphenylphosphine (TPP) treated graphene was −57 V, which provided clear evidence of n-type doping. • Substitutional doping of graphene with phosphorus is verified by the XPS spectra of P 2p core level and EELS mapping of phosphorus. • The chemical bonding between P and graphene is very stable for a long time in air (2 months). - Abstract: Graphene is considered a host material for various applications in next-generation electronic devices. However, despite its excellent properties, one of the most important issues to be solved as an electronic material is the creation of an energy band gap. Substitution doping is a promising method for opening the energy band gap of graphene. Herein, we demonstrate the substitutional doping of graphene with phosphorus using inductively coupled plasma (ICP) and triphenylphosphine (TPP) treatments. The electrical transfer characteristics of the phosphorus doped graphene field effect transistor (GFET) have a V{sub dirac} of ∼ − 54 V. The chemical bonding between P and C was clearly observed in XPS spectra, and uniform distribution of phosphorus within graphene domains was confirmed by EELS mapping. The capability for substitutional doping of graphene with phosphorus can significantly promote the development of graphene based electronic devices.

Kinetic energy and charge distributions of multiply charged ions produced by heavy ions and by synchrotron radiation

International Nuclear Information System (INIS)

Levin, J.C.; Biedermann, C.; Cederquist, H.; Liljeby, L.; Short, R.T.; Sellin, I.A.

1989-01-01

This paper contrasts two methods of production of multiply charged ions which may have application in future hot-atom chemistry experiments. Interest in extending the study of ion-atom collisions from MeV to keV to eV energies has grown rapidly in the last decade as previously inaccessible astrophysical, fusion, and spectroscopic problems have been addressed. One of these methods involves highly charged secondary beams formed from ions created in dilute gas samples irradiated by fast (MeV), high-charge-state, heavy ions. The measurements show, however, that such ions often have mean recoil energies two orders of magnitude higher than kinetic energies of ions in similar charge states resulting from vacancy cascades of atomic inner shells photoionized by synchrotron x rays. These results may be applicable to development of a cold source of highly charged ions featuring low energy spread and good angular definition. Results from other laboratories (Grandin et al at Ganil, Ullrich et al in Frankfurt, and Watson et al at Texas A ampersand M) will also be discussed

Theoretical evaluation of high-energy lithium metal phosphate cathode materials in Li-ion batteries

Science.gov (United States)

Howard, Wilmont F.; Spotnitz, Robert M.

Lithium metal phosphates (olivines) are emerging as long-lived, safe cathode materials in Li-ion batteries. Nano-LiFePO 4 already appears in high-power applications, and LiMnPO 4 development is underway. Current and emerging Fe- and Mn-based intercalants, however, are low-energy producers compared to Ni and Co compounds. LiNiPO 4, a high voltage olivine, has the potential for superior energy output (>10.7 Wh in 18650 batteries), compared with commercial Li(Co,Ni)O 2 derivatives (up to 9.9 Wh). Speculative Co and Ni olivine cathode materials charged to above 4.5 V will require significant advances in electrolyte compositions and nanotechnology before commercialization. The major drivers toward 5 V battery chemistries are the inherent abuse tolerance of phosphates and the economic benefit of LiNiPO 4: it can produce 34% greater energy per dollar of cell material cost than LiAl 0.05Co 0.15Ni 0.8O 2, today's "standard" cathode intercalant in Li-ion batteries.

Laser thermal annealing of Ge, optimized for highly activated dopants and diode ION/IOFF ratios

DEFF Research Database (Denmark)

Shayesteh, M.; O'Connell, D.; Gity, F.

2014-01-01

The authors compared the influence of laser thermal annealing (LTA) and rapid thermal annealing (RTA) on dopant activation and electrical performance of phosphorus and arsenic doped n+/p junction. High carrier concentration above 1020 cm-3 as well as an ION/IOFF ratio of approximately 105 and ide...

Experimental study of interactions of highly charged ions with atoms at keV energies: Progress report for period May 15, 1985-February 15, 1987

International Nuclear Information System (INIS)

Kostroun, V.O.

1987-01-01

Interest in interactions of low energy highly charged ions with electrons, atoms or ions is due to their importance to controlled thermonuclear fusion research and the interesting nature of the fundamental processes involved. Studies of such interactions have long been hampered by a lack of suitable ions sources. A superconducting solenoid, cryogenic Electron Beam Ion Source, CEBIS, has been constructed at Cornell University to produce low energy very highly charged ions. At present, using a pulsed 0.5A,8.5 keV electron beam, the source is capable of producing highly charged ions of C,N,O, including bare nuclei, and ions of Ar up to charge state 11 + in 1 millisecond of confinement time. The source is being used in experiments to investigate charge transfer and accompanying processes in low energy, highly charged ion-atom collisions

Ion-induced particle desorption in time-of-flight medium energy ion scattering

Science.gov (United States)

Lohmann, S.; Primetzhofer, D.

2018-05-01

Secondary ions emitted from solids upon ion impact are studied in a time-of-flight medium energy ion scattering (ToF-MEIS) set-up. In order to investigate characteristics of the emission processes and to evaluate the potential for surface and thin film analysis, experiments employing TiN and Al samples were conducted. The ejected ions exhibit a low initial kinetic energy of a few eV, thus, requiring a sufficiently high acceleration voltage for detection. Molecular and atomic ions of different charge states originating both from surface contaminations and the sample material are found, and relative yields of several species were determined. Experimental evidence that points towards a predominantly electronic sputtering process is presented. For emitted Ti target atoms an additional nuclear sputtering component is suggested.

HITRAP: A Facility for Experiments with Trapped Highly Charged Ions

International Nuclear Information System (INIS)

Quint, W.; Dilling, J.; Djekic, S.; Haeffner, H.; Hermanspahn, N.; Kluge, H.-J.; Marx, G.; Moore, R.; Rodriguez, D.; Schoenfelder, J.; Sikler, G.; Valenzuela, T.; Verdu, J.; Weber, C.; Werth, G.

2001-01-01

HITRAP is a planned ion trap facility for capturing and cooling of highly charged ions produced at GSI in the heavy-ion complex of the UNILAC-SIS accelerators and the ESR storage ring. In this facility heavy highly charged ions up to uranium will be available as bare nuclei, hydrogen-like ions or few-electron systems at low temperatures. The trap for receiving and studying these ions is designed for operation at extremely high vacuum by cooling to cryogenic temperatures. The stored highly charged ions can be investigated in the trap itself or can be extracted from the trap at energies up to about 10 keV/q. The proposed physics experiments are collision studies with highly charged ions at well-defined low energies (eV/u), high-accuracy measurements to determine the g-factor of the electron bound in a hydrogen-like heavy ion and the atomic binding energies of few-electron systems, laser spectroscopy of HFS transitions and X-ray spectroscopy

A high energy and power sodium-ion hybrid capacitor based on nitrogen-doped hollow carbon nanowires anode

Science.gov (United States)

Li, Dongdong; Ye, Chao; Chen, Xinzhi; Wang, Suqing; Wang, Haihui

2018-04-01

The sodium ion hybrid capacitor (SHC) has been attracting much attention. However, the SHC's power density is significantly confined to a low level due to the sluggish ion diffusion in the anode. Herein, we propose to use an electrode with a high double layer capacitance as the anode in the SHC instead of insertion anodes. To this aim, nitrogen doped hollow carbon nanowires (N-HCNWs) with a high specific surface area are prepared, and the high capacitive contribution during the sodium ion storage process is confirmed by a series of electrochemical measurements. A new SHC consisting of a N-HCNW anode and a commercial active carbon (AC) cathode is fabricated for the first time. Due to the hybrid charge storage mechanism combining ion insertion and capacitive process, the as-fabricated SHC strikes a balance between the energy density and power density, a energy density of 108 Wh kg-1 and a power density of 9 kW kg-1 can be achieved, which overwhelms the electrochemical performances of most reported AC-based SHCs.

High energy ions and energetic plasma irradiation effects on aluminum in a Filippov-type plasma focus

Energy Technology Data Exchange (ETDEWEB)

Roshan, M.V. [National Institute of Education, Nanyang Technological University, 1 Nanyang Walk, Singapore 637616 (Singapore)], E-mail: mroshan20@yahoo.com; Rawat, R.S. [National Institute of Education, Nanyang Technological University, 1 Nanyang Walk, Singapore 637616 (Singapore); Babazadeh, A.R.; Emami, M.; Sadat Kiai, S.M. [Plasma Physics Research Center, AEOI, 14155-1339 Tehran (Iran, Islamic Republic of); Verma, R.; Lin, J.J.; Talebitaher, A.R.; Lee, P.; Springham, S.V. [National Institute of Education, Nanyang Technological University, 1 Nanyang Walk, Singapore 637616 (Singapore)

2008-12-30

High energy ions and energetic plasma irradiation of aluminum cathode inserts have been accomplished in nitrogen and argon filled plasma focus device. The Filippov-type plasma focus facility, Dena, with 288 {mu}F capacitor bank and charging voltage of 25 kV (90 kJ maximum storage energy) was first optimized for strong ion beam generation for nitrogen and argon gases by maximizing hard X-ray emission efficiency. X-ray diffraction analysis as well as scanning electron microscopy along with energy dispersive X-ray spectroscopy carried out to study the structural, morphological and compositional profile of the treated samples. Change in preferred orientation, emergence of meta-stable phases, generation of copper micro-droplets, and production of cracks across the sample are demonstrated and discussed. The micro-hardness measurements in Vickers scale reveal that after ion irradiation, the surface hardness of samples is reduced.

Li-Ion, Ultra-capacitor Based Hybrid Energy Module

National Research Council Canada - National Science Library

Daboussi, Zaher; Paryani, Anil; Khalil, Gus; Catherino, Henry; Gargies, Sonya

2007-01-01

.... To determine the optimum utilization of ultra-capacitors in applications where high power density and high energy density are required, an optimized Li-Ion/Ultra-capacitor Hybrid Energy Module (HEM...

The prospect for fusion energy with light ions

International Nuclear Information System (INIS)

Mehlhorn, T.A.; Adams, R.G.; Bailey, J.E.

1998-01-01

Intense ion beams may be the best option for an Inertial Fusion Energy (IFE) driver. While light ions may be the long-term pulsed power approach to IFE, the current economic climate is such that there is no urgency in developing fusion energy sources. Research on light ion beams at Sandia will be suspended at the end of this fiscal year in favor of z-pinches studying ICF target physics, high yield fusion, and stewardship issues. The authors document the status of light ion research and the understanding of the feasibility of scaling light ions to IFE

Vacancy supersaturations produced by high-energy ion implantation

International Nuclear Information System (INIS)

Venezia, V.C.; Eaglesham, D.J.; Jacobson, D.C.; Gossmann, H.J.

1998-01-01

A new technique for detecting the vacancy clusters produced by high-energy ion implantation into silicon is proposed and tested. This technique takes advantage of the fact that metal impurities, such as Au, are gettered near one-half of the projected range (1/2 R p ) of MeV implants. The vacancy clustered region produced by a 2 MeV Si + implant into silicon has been labeled with Au diffused in from the front surface. The trapped Au was detected by Rutherford backscattering spectrometry (RBS) to profile the vacancy clusters. Cross section transmission electron microscopy (XTEM) analysis shows that the Au in the region of vacancy clusters is in the form of precipitates. By annealing MeV implanted samples prior to introduction of the Au, changes in the defect concentration within the vacancy clustered region were monitored as a function of annealing conditions

New 2-stage ion microprobes and a move to higher energies

Energy Technology Data Exchange (ETDEWEB)

Legge, G.J.F.; Dymnikov, A.; Moloney, G.; Saint, A. [Melbourne Univ., Parkville, VIC (Australia). School of Physics; Cohen, D. [Australian Nuclear Science and Technology Organisation, Lucas Heights, NSW (Australia)

1996-12-31

Recent moves in Ion Beam Microanalysis towards the use of a rapidly growing number of very high resolution, low current and single ion techniques has led to the need for high demagnification and greatly improved beam quality. There is also a move to apply Microbeams at higher energies and with heavier ions. This also puts demands on the focusing system and beam control. This paper describes the recent development of 2-stage lens systems to be applied here and overseas, both at very high resolution and at high energies with heavy ions. It looks at new ion beam analysis applications of such ion microprobes. 8 refs., 1 tab., 1 fig.

New 2-stage ion microprobes and a move to higher energies

Energy Technology Data Exchange (ETDEWEB)

Legge, G J.F.; Dymnikov, A; Moloney, G; Saint, A [Melbourne Univ., Parkville, VIC (Australia). School of Physics; Cohen, D [Australian Nuclear Science and Technology Organisation, Lucas Heights, NSW (Australia)

1997-12-31

Recent moves in Ion Beam Microanalysis towards the use of a rapidly growing number of very high resolution, low current and single ion techniques has led to the need for high demagnification and greatly improved beam quality. There is also a move to apply Microbeams at higher energies and with heavier ions. This also puts demands on the focusing system and beam control. This paper describes the recent development of 2-stage lens systems to be applied here and overseas, both at very high resolution and at high energies with heavy ions. It looks at new ion beam analysis applications of such ion microprobes. 8 refs., 1 tab., 1 fig.

Study of the effects of focused high-energy boron ion implantation in diamond

Science.gov (United States)

Ynsa, M. D.; Agulló-Rueda, F.; Gordillo, N.; Maira, A.; Moreno-Cerrada, D.; Ramos, M. A.

2017-08-01

Boron-doped diamond is a material with a great technological and industrial interest because of its exceptional chemical, physical and structural properties. At modest boron concentrations, insulating diamond becomes a p-type semiconductor and at higher concentrations a superconducting metal at low temperature. The most conventional preparation method used so far, has been the homogeneous incorporation of boron doping during the diamond synthesis carried out either with high-pressure sintering of crystals or by chemical vapour deposition (CVD) of films. With these methods, high boron concentration can be included without distorting significantly the diamond crystalline lattice. However, it is complicated to manufacture boron-doped microstructures. A promising alternative to produce such microstructures could be the implantation of focused high-energy boron ions, although boron fluences are limited by the damage produced in diamond. In this work, the effect of focused high-energy boron ion implantation in single crystals of diamond is studied under different irradiation fluences and conditions. Micro-Raman spectra of the sample were measured before and after annealing at 1000 °C as a function of irradiation fluence, for both superficial and buried boron implantation, to assess the changes in the diamond lattice by the creation of vacancies and defects and their degree of recovery after annealing.

Discussion of electron capture theories for ion-atom collisions at high energies

Energy Technology Data Exchange (ETDEWEB)

Miraglia, J E [Instituto de Astronomia y Fisica del Espacio, Buenos Aires (Argentina); Piacentini, R D [Consejo Nacional de Investigaciones Cientificas y Tecnicas, Buenos Aires (Argentina); Rivarola, R D [Rosario Univ. Nacional (Argentina). Dept. de Fisica; Salin, A [Bordeaux-1 Univ., 33 - Talence (France)

1981-03-14

Different theories of charge exchange processes in ion-atom collisions at high energies for the H/sup +/-H system are considered. Large discrepancies are found in the differential cross sections obtained from the various models. The validity of Dettmann's peaking approximation is analysed by comparison with exact values for the first- and second-order Oppenheimer-Brinkman-Kramers (OBK 1 and OBK 2) theories. It is also shown that for energies up to a few MeV the OBK 2 differential cross sections are higher than the corresponding OBK 1 ones. Total cross sections in the OBK 2 approximation are given.

Low-energy ion beam extraction and transport: Experiment--computer comparison

International Nuclear Information System (INIS)

Spaedtke, P.; Brown, I.; Fojas, P.

1994-01-01

Ion beam formation at low energy (∼1 keV or so) is more difficult to accomplish than at high energy because of beam blowup by space-charge forces in the uncompensated region within the extractor, an effect which is yet more pronounced for heavy ions and for high beam current density. For the same reasons, the extracted ion beam is more strongly subject to space charge blowup than higher energy beams if it is not space-charge neutralized to a high degree. A version of vacuum arc ion source with an extractor that produces low-energy metal ion beams at relatively high current (∼0.5--10 kV at up to ∼100 mA) using a multi-aperture, accel--decel extractor configuration has been created. The experimentally observed beam extraction characteristics of this source is compared with those predicted using the AXCEL-INP code, and the implied downstream beam transport with theoretical expectations. It is concluded that the low-energy extractor performance is in reasonable agreement with the code, and that good downstream space charge neutralization is obtained. Here, the code and the experimental results are described, and the features that contribute to good low-energy performance are discussed

Effect of energy selection on quantitative analysis in secondary ion microanalysis

International Nuclear Information System (INIS)

Steele, I.M.; Solberg, T.N.; Smith, J.V.; Clayton, R.N.; Hutcheon, I.D.

1977-01-01

Systematic change of voltage on the components of the secondary ion (SI) extraction system of our AEI-IM20 ion microprobe produced major changes of relative intensities of secondary ions passing through the mass spectrometer. The repeller, which bends the SI beam through about 60 0 , has the greatest effect, and can be used to plot the energy distribution. The extractor and the deflecting and focusing components have smaller but significant effects. Because low-energy secondary ions have a near-symmetrical distribution, whereas high-energy ones have an assymetric distribution favoring high energies, tuning of the acceptance band to higher energy reduces interference from low-energy ions, which tend to be unwanted molecular ions, at the expense of reduced transmission. Tuning to lower energy increases interference but gives higher transmission. The former condition is desirable for instruments restricted to low mass resolution, whereas both conditions are valuable for instruments adjustable for both high and low mass resolution. Other important factors are (a) sensitivity to surface irregularities which perturb SI energy collection, and (b) change in derived 'temperatures' from thermodynamic sputtering models merely from tuning the energy acceptance band. Careful attention to the above factors yielded reproducible SI ratios for the binary series of plagioclase feldspars. (Auth.)

Spectroscopy of highly charged tungsten ions with Electron Beam Ion Traps

International Nuclear Information System (INIS)

Sakaue, Hiroyuki A.; Kato, Daiji; Morita, Shigeru; Murakami, Izumi; Yamamoto, Norimasa; Ohashi, Hayato; Yatsurugi, Junji; Nakamura, Nobuyuki

2013-01-01

We present spectra of highly charged tungsten ions in the extreme ultra-violet (EUV) by using electron beam ion traps. The electron energy dependence of spectra is investigated of electron energies from 490 to 1440 eV. Previously unreported lines are presented in the EUV range, and some of them are identified by comparing the wavelengths with theoretical calculations. (author)

The measurements of light high-energy ions in NINA-2 experiment

Directory of Open Access Journals (Sweden)

A. Leonov

2007-10-01

Full Text Available The flux of energetic light ions at low altitude is both an important input and output for self-consistent calculations of albedo particles resulting from the interaction of trapped and cosmic ray particles, with the upper atmosphere. In addition, data on the flux of light ions are needed to evaluate radiation damages on space-borne instruments and on space mission crews. In spite of that, sources of data on the flux of energetic ions at LEO are roughly limited to the AP-8 model, CREME/CREME96 codes and the SAMPEX, NOAA/TIROS satellites. The existing and operational European SAC-C/ICARE and PROBA-1/SREM instruments could also be potential sources for proton data at LEO. Although AP-8 and SAMPEX/PSB97 may be publicly accessed through the SPENVIS, they exhibit an order of magnitude difference in low altitude proton fluxes and they do not contain helium fluxes. Therefore, improved light ion radiation models are still needed.

In this paper we present a procedure to identify and measure the energy of ions that are not stopped in the NINA-2 instrument. Moreover, problems related to particles that cross the instrument in the opposite direction are addressed and shown to be a possible cause of particle misidentification. Measuring fluxes of low abundance elements like energetic helium ions requires a good characterisation of all possible sources of backgrounds in the detector. Hints to determine the several contributions to the background are presented herein and may be applied to extract an order of magnitude of energetic ions fluxes from existing data sets, while waiting for dedicated high performance instruments.

The measurements of light high-energy ions in NINA-2 experiment

Directory of Open Access Journals (Sweden)

A. Leonov

2007-10-01

Full Text Available The flux of energetic light ions at low altitude is both an important input and output for self-consistent calculations of albedo particles resulting from the interaction of trapped and cosmic ray particles, with the upper atmosphere. In addition, data on the flux of light ions are needed to evaluate radiation damages on space-borne instruments and on space mission crews. In spite of that, sources of data on the flux of energetic ions at LEO are roughly limited to the AP-8 model, CREME/CREME96 codes and the SAMPEX, NOAA/TIROS satellites. The existing and operational European SAC-C/ICARE and PROBA-1/SREM instruments could also be potential sources for proton data at LEO. Although AP-8 and SAMPEX/PSB97 may be publicly accessed through the SPENVIS, they exhibit an order of magnitude difference in low altitude proton fluxes and they do not contain helium fluxes. Therefore, improved light ion radiation models are still needed. In this paper we present a procedure to identify and measure the energy of ions that are not stopped in the NINA-2 instrument. Moreover, problems related to particles that cross the instrument in the opposite direction are addressed and shown to be a possible cause of particle misidentification. Measuring fluxes of low abundance elements like energetic helium ions requires a good characterisation of all possible sources of backgrounds in the detector. Hints to determine the several contributions to the background are presented herein and may be applied to extract an order of magnitude of energetic ions fluxes from existing data sets, while waiting for dedicated high performance instruments.

Single ion induced surface nanostructures: a comparison between slow highly charged and swift heavy ions.

Science.gov (United States)

Aumayr, Friedrich; Facsko, Stefan; El-Said, Ayman S; Trautmann, Christina; Schleberger, Marika

2011-10-05

This topical review focuses on recent advances in the understanding of the formation of surface nanostructures, an intriguing phenomenon in ion-surface interaction due to the impact of individual ions. In many solid targets, swift heavy ions produce narrow cylindrical tracks accompanied by the formation of a surface nanostructure. More recently, a similar nanometric surface effect has been revealed for the impact of individual, very slow but highly charged ions. While swift ions transfer their large kinetic energy to the target via ionization and electronic excitation processes (electronic stopping), slow highly charged ions produce surface structures due to potential energy deposited at the top surface layers. Despite the differences in primary excitation, the similarity between the nanostructures is striking and strongly points to a common mechanism related to the energy transfer from the electronic to the lattice system of the target. A comparison of surface structures induced by swift heavy ions and slow highly charged ions provides a valuable insight to better understand the formation mechanisms. © 2011 IOP Publishing Ltd

Importance of ion energy on SEU in CMOS SRAMs

Energy Technology Data Exchange (ETDEWEB)

Dodd, P.E.; Shaneyfelt, M.R.; Sexton, F.W.; Hash, G.L.; Winokur, P.S. [Sandia National Labs., Albuquerque, NM (United States); Musseau, O.; Leray, J.L. [CEA-DAM, Bruyeres-le-Chatel (France)

1998-03-01

The single-event upset (SEU) responses of 16 Kbit to 1 Mbit SRAMs irradiated with low and high-energy heavy ions are reported. Standard low-energy heavy ion tests appear to be sufficiently conservative for technologies down to 0.5 {micro}m.

Metabolic factors affecting enhanced phosphorus uptake by activated sludge.

Science.gov (United States)

Boughton, W H; Gottfried, R J; Sinclair, N A; Yall, I

1971-10-01

Activated sludges obtained from the Rilling Road plant located at San Antonio, Tex., and from the Hyperion treatment plant located at Los Angeles, Calif., have the ability to remove all of the orthophosphate normally present in Tucson sewage within 3 hr after being added to the waste water. Phosphorus removal was independent of externally supplied sources of energy and ions, since orthophosphate and (32)P radioactivity were readily removed from tap water, glass-distilled water, and deionized water. Phosphorus uptake by Rilling sludge in the laboratory appears to be wholly biological, as it has an optimum pH range (7.7 to 9.7) and an optimum temperature range (24 to 37 C). It was inhibited by HgCl(2), iodoacetic acid, p-chloromercuribenzoic acid, NaN(3), and 2, 4-dinitrophenol (compounds that affect bacterial membrane permeability, sulfhydryl enzymes, and adenosine triphosphate synthesis). Uptake was inhibited by 1% NaCl but was not affected by 10(-3)m ethylenediaminetetraacetic acid disodium salt (a chelating agent for many metallic ions).

Monte Carlo simulation for neutron yield produced by bombarding thick targets with high energy heavy ions

Energy Technology Data Exchange (ETDEWEB)

Oranj, Leila Mokhtari; Oh, Joo Hee; Yoon, Moo Hyun; Lee, Hee Seock [POSTECH, Pohang (Korea, Republic of)

2013-04-15

One of radiation shielding issues at heavy-ion accelerator facilities is to estimate neutron production by primary heavy ions. A few Monte Carlo transport codes such as FLUKA and PHITS can work with primary heavy ions. Recently IBS/RISP((Rare Isotope Science Project) started to design a high-energy, high-power rare isotope accelerator complex for nuclear physics, medical and material science and applications. There is a lack of experimental and simulated data about the interaction of major beam, {sup 238}U with materials. For the shielding design of the end of first accelerating section section, we calculate a differential neutron yield using the FLUKA code for the interaction of 18.5 MeV/u uranium ion beam with thin carbon stripper of 1.3 μm). The benchmarking studies were also done to prove the yield calculation for 400 MeV/n {sup 131}Xe and other heavy ions. In this study, the benchmarking for Xe-C, Xe-Cu, Xe-Al, Xe-Pb and U-C, other interactions were performed using the FLUKA code. All of results show that the FLUKA can evaluate the heavy ion induced reaction with good uncertainty. For the evaluation of neutron source term, the calculated neutron yields are shown in Fig. 2. The energy of Uranium ion beam is only 18.5 MeV/u, but the energy of produced secondary neutrons was extended over 100 MeV. So the neutron shielding and the damage by those neutrons is expected to be serious. Because of thin stripper, the neutron intensity at forward direction was high. But the the intensity of produced secondary photons was relatively low and mostly the angular property was isotropic. For the detail shielding design of stripper section of RISP rare istope accelerator, the benchmarking study and preliminary evaluation of neutron source term from uranium beam have been carried out using the FLUKA code. This study is also compared with the evaluation results using the PHITS code performed coincidently. Both studies shows that two monte carlo codes can give a good results for

Coulomb-driven energy boost of heavy ions for laser-plasma acceleration.

Science.gov (United States)

Braenzel, J; Andreev, A A; Platonov, K; Klingsporn, M; Ehrentraut, L; Sandner, W; Schnürer, M

2015-03-27

An unprecedented increase of kinetic energy of laser accelerated heavy ions is demonstrated. Ultrathin gold foils have been irradiated by an ultrashort laser pulse at a peak intensity of 8×10^{19}  W/  cm^{2}. Highly charged gold ions with kinetic energies up to >200  MeV and a bandwidth limited energy distribution have been reached by using 1.3 J laser energy on target. 1D and 2D particle in cell simulations show how a spatial dependence on the ion's ionization leads to an enhancement of the accelerating electrical field. Our theoretical model considers a spatial distribution of the ionization inside the thin target, leading to a field enhancement for the heavy ions by Coulomb explosion. It is capable of explaining the energy boost of highly charged ions, enabling a higher efficiency for the laser-driven heavy ion acceleration.

Electronic excitation effects on secondary ion emission in highly charged ion-solid interaction

International Nuclear Information System (INIS)

Sekioka, T.; Terasawa, M.; Mitamura, T.; Stoeckli, M.P.; Lehnert, U.; Fehrenbach, C.

2001-01-01

In order to investigate the secondary ion emission from the surface of conductive materials bombarded by highly charged heavy ions, we have done two types of experiments. First, we have measured the yield of the sputtered ions from the surface of solid targets of conductive materials (Al, Si, Ni, Cu) bombarded by Xe q+ (q=15-44) at 300 keV (v p =0.30 a.u) and at 1.0 MeV (v p =0.54 a.u). In view of the secondary ion yields as a function of the potential energy of the projectile, the increase rates below q=35, where the potential energy amounts to 25.5 keV, were rather moderate and showed a prominent increase above q=35. These phenomena were rather strong in the case of the metal targets. Second, we have measured the energy dependence of the yield of the sputtered ions from the surface of solid targets of conductive materials (C, Al) bombarded by Xe q+ (q=30,36,44) between 76 keV (v p =0.15 a.u) and 6.0 MeV (v p =1.3 a.u). A broad enhancement of the secondary ion yield has been found for Al target bombarded by Xe 44+ . From these experimental results, the electronic excitation effects in conductive materials for impact of slow highly charged heavy ions bearing high potential energy is discussed

Biomaterial imaging with MeV-energy heavy ion beams

Energy Technology Data Exchange (ETDEWEB)

Seki, Toshio, E-mail: seki@sakura.nucleng.kyoto-u.ac.jp [Department of Nuclear Engineering, Kyoto Univ., Uji, Kyoto 611-0011 (Japan); CREST, Japan Science and Technology Agency (JST), Chiyoda, Tokyo 102-0075 (Japan); Wakamatsu, Yoshinobu; Nakagawa, Shunichiro [Department of Nuclear Engineering, Kyoto Univ., Uji, Kyoto 611-0011 (Japan); Aoki, Takaaki [Department of Electronic Science and Engineering, Kyoto Univ., Nishikyo, Kyoto 615-8510 (Japan); CREST, Japan Science and Technology Agency (JST), Chiyoda, Tokyo 102-0075 (Japan); Ishihara, Akihiko [Laboratory of Cell Biology and Life Science, Graduate School of Human and Environmental Studies, Kyoto Univ., Sakyo, Kyoto 606-8501 (Japan); Matsuo, Jiro [Quantum Science and Engineering Center, Kyoto Univ., Uji, Kyoto 611-0011 (Japan); CREST, Japan Science and Technology Agency (JST), Chiyoda, Tokyo 102-0075 (Japan)

2014-08-01

The spatial distribution of several chemical compounds in biological tissues and cells can be obtained with mass spectrometry imaging (MSI). In conventional secondary ion mass spectrometry (SIMS) with keV-energy ion beams, elastic collisions occur between projectiles and atoms of constituent molecules. The collisions produce fragments, making the acquisition of molecular information difficult. In contrast, ion beams with MeV-energy excite near-surface electrons and enhance the ionization of high-mass molecules; hence, SIMS spectra of fragment-suppressed ionized molecules can be obtained with MeV-SIMS. To compare between MeV and conventional SIMS, we used the two methods based on MeV and Bi{sub 3}-keV ions, respectively, to obtain molecular images of rat cerebellum. Conventional SIMS images of m/z 184 were clearly observed, but with the Bi{sub 3} ion, the distribution of the molecule with m/z 772.5 could be observed with much difficulty. This effect was attributed to the low secondary ion yields and we could not get many signal counts with keV-energy beam. On the other hand, intact molecular ion distributions of lipids were clearly observed with MeV-SIMS, although the mass of all lipid molecules was higher than 500 Da. The peaks of intact molecular ions in MeV-SIMS spectra allowed us to assign the mass. The high secondary ion sensitivity with MeV-energy heavy ions is very useful in biomaterial analysis.

Biomaterial imaging with MeV-energy heavy ion beams

International Nuclear Information System (INIS)

Seki, Toshio; Wakamatsu, Yoshinobu; Nakagawa, Shunichiro; Aoki, Takaaki; Ishihara, Akihiko; Matsuo, Jiro

2014-01-01

The spatial distribution of several chemical compounds in biological tissues and cells can be obtained with mass spectrometry imaging (MSI). In conventional secondary ion mass spectrometry (SIMS) with keV-energy ion beams, elastic collisions occur between projectiles and atoms of constituent molecules. The collisions produce fragments, making the acquisition of molecular information difficult. In contrast, ion beams with MeV-energy excite near-surface electrons and enhance the ionization of high-mass molecules; hence, SIMS spectra of fragment-suppressed ionized molecules can be obtained with MeV-SIMS. To compare between MeV and conventional SIMS, we used the two methods based on MeV and Bi 3 -keV ions, respectively, to obtain molecular images of rat cerebellum. Conventional SIMS images of m/z 184 were clearly observed, but with the Bi 3 ion, the distribution of the molecule with m/z 772.5 could be observed with much difficulty. This effect was attributed to the low secondary ion yields and we could not get many signal counts with keV-energy beam. On the other hand, intact molecular ion distributions of lipids were clearly observed with MeV-SIMS, although the mass of all lipid molecules was higher than 500 Da. The peaks of intact molecular ions in MeV-SIMS spectra allowed us to assign the mass. The high secondary ion sensitivity with MeV-energy heavy ions is very useful in biomaterial analysis

Ion energy/momentum effects during ion assisted growth of niobium nitride films

Science.gov (United States)

Klingenberg, Melissa L.

The research described herein was performed to better understand and discern ion energy vs. ion momentum effects during ion beam assisted (IBAD) film growth and their effects on residual stress, crystalline structure, morphology, and composition, which influence film tribological properties. NbxN y was chosen for this research because it is a refractory material that can possess a large number of crystalline structures, and it has been found to have good tribological properties. To separate the effects of momentum transfer per arriving atom (p/a), which considers bombarding species mass, energy, and ion-to-atom transport ratio, from those of energy deposition per arriving atom (E/a), a mass independent parameter, different inert ion beams (krypton, argon, and neon) were used to create a matrix of coatings formed using similar energy deposition, but different momentum transfer and vice versa. Deposition was conducted in a research-scale IBAD system using electron beam evaporation, a radio frequency ion source, and a neutral nitrogen gas backfill. Films were characterized using x-ray diffraction, atomic force microscopy, Rutherford backscattering spectrometry, and residual stress analysis. Direct and quantifiable effects of bombardment were observed; however, energy deposition and momentum transfer effects could not be completely separated, confirming that thin film processes are complex. Complexities arose from ion-specific interactions (ion size, recoil energy, per cent reflected neutrals, Penning ionization, etc.) and chemistry effects that are not considered by the simple models. Overall, it can be stated that bombardment promoted nitride formation, nanocrystallinity, and compressive stress formation; influenced morphology (which influenced post-deposition oxygen uptake) and stress evolution; increased lattice parameter; modified crystalline phase and texture; and led to inert gas incorporation. High stress levels correlated strongly with material disorder and

Phosphorus and groundwater: Establishing links between agricultural use and transport to streams

Science.gov (United States)

Domagalski, Joseph L.; Johnson, Henry

2012-01-01

Phosphorus is a highly reactive element that is essential for life and forms a variety of compounds in terrestrial and aquatic ecosystems. In water, phosphorus may be present as the orthophosphate ion (PO43-) and is also present in all life forms as an essential component of cellular material. In natural ecosystems, phosphorus is derived from the erosion of rocks and is conserved for plant growth as it is returned to the soil through animal waste and the decomposition of plant and animal tissue; but in agricultural systems, a portion of the phosphorus is removed with each harvest, especially since phosphorus is concentrated in the seeds and fruit. Phosphorus is added to soil by using chemical fertilizers, manure, and composted materials. Agricultural use of chemical phosphorus fertilizer, in the United States, in 2008 was 4,247,000 tons, which is an increase of 25 percent since 1964 (http://www.ers.usda.gov/Data/FertilizerUse/). Widely grown corn, soybeans, and wheat use the greatest amount of phosphorus fertilizer among agricultural crops.

Final Report - Advanced High Energy Li-Ion Cell for PHEV and EV Applications

Energy Technology Data Exchange (ETDEWEB)

Singh, Jagat [3M Company, Maplewood, MN (United States)

2017-03-22

Lithium Ion Battery (LIB) technology’s potential to enable a commercially viable high energy density is the key to a lower $/Wh, thereby a low cost battery. The design of a LIB with high energy, high power, safety and long life is a challenge that requires cell design from the ground up and synergy between all components. 3M Company (3M), the Recipient, led by its Principal Investigator, Jagat Singh, pursued this challenging task of a LIB by ‘teaming’ key commercial businesses [General Motors (GM), Umicore and Iontensity] and labs [Army Research Laboratory (ARL) and Lawrence Berkley National Laboratory (LBNL)]. The technology from each team member was complimentary and a close working relationship spanning the value chain drove productivity.The completion of this project is a significant step towards more energy efficient and environmentally friendly vehicles, making America less dependent on imported oil.

High dose radiation damage in nuclear energy structural materials investigated by heavy ion irradiation simulation

International Nuclear Information System (INIS)

Zheng Yongnan; Xu Yongjun; Yuan Daqing

2014-01-01

Structural materials in ITER, ADS and fast reactor suffer high dose irradiations of neutrons and/or protons, that leads to severe displacement damage up to lOO dpa per year. Investigation of radiation damage induced by such a high dose irradiation has attracted great attention along with the development of nuclear energy facilities of new generation. However, it is deeply hampered for the lacking of high dose neutron and proton sources. Irradiation simulation of heavy ions produced by accelerators opens up an effective way for laboratory investigation of high dose irradiation induced radiation damage encountered in the ITER, ADS, etc. Radiation damage is caused mainly by atomic displacement in materials. The displacement rate of heavy ions is about lO 3 ∼10 7 orders higher than those of neutrons and protons. High displacement rate of heavy ions significantly reduces the irradiation time. The heavy ion irradiation simulation technique (HIIS) technique has been developed at China Institute of Atomic Energy and a series of the HIIS experiments have been performed to investigate radiation damage in stainless steels, tungsten and tantalum at irradiation temperatures from room temperature to 800 ℃ and in the irradiation dose region up to 100 dpa. The experimental results show that he radiation swelling peak for the modified stainless steel appears in the temperature region around 580 ℃ and the radiation damage is more sensitive to the temperature, the size of the radiation induced vacancy cluster or void increase with the increasing of the irradiation dose, and among the three materials the home-made modified stainless steel has the best radiation resistant property. (authors)

EUV spectrum of highly charged tungsten ions in electron beam ion trap

International Nuclear Information System (INIS)

Sakaue, H.A.; Kato, D.; Murakami, I.; Nakamura, N.

2016-01-01

We present spectra of highly charged tungsten ions in the extreme ultra-violet (EUV) by using electron beam ion traps. The electron energy dependence of spectra was investigated for electron energy from 540 to 1370 eV. Previously unreported lines were presented in the EUV range, and comparing the wavelengths with theoretical calculations identified them. (author)

The present state and perspectives of low-energy heavy ion biology

International Nuclear Information System (INIS)

Yuan Chengling; Yu Zengliang

2004-01-01

The interaction between low-energy ions and matter has been concerned rarely comparing to that of high-energy ions. It is even more unusual to find studies of the interaction of low-energy ions and complicated organisms. However, the discovery of bioeffects induced by ion beam implantation has opened a new branch in the field of ion beam applications in the life science--Low-energy Heavy Ion Biology. The mutagenic effect of low energy heavy ions was firstly reported in 1986 in rice. Since then, a damage mechanism involved in energy absorption, mass deposition, and charge exchange has been proposed. Accumulating evidence has indicated that these three factors are key determinants in the bioeffects induced by low energy heavy ions, which has opened new opportunities for mutational breeding, gene transferring, cell modification, and cell fusion. In recent years, the ion beam implantation technique has been widely applied in many fields, and increasing research interest in the field has been seen. The authors summarize recent advances in research on the role of low-energy ions in terms of the mechanisms and applications

Single-walled carbon nanotubes as stabilizing agents in red phosphorus Li-ion battery anodes

KAUST Repository

Smajic, Jasmin

2017-08-16

Phosphorus boasts extremely high gravimetric and volumetric capacities but suffers from poor electrochemical stability with significant capacity loss immediately after the first cycle. We propose to circumvent this issue by mixing amorphous red phosphorus with single-walled carbon nanotubes. Employing a non-destructive sublimation–deposition method, we have synthesized composites where the synergetic effect between red phosphorus and single-walled carbon nanotubes allows for a considerable improvement in the electrochemical stability of battery anodes. In contrast to the average 40% loss of capacity after 50 cycles for other phosphorus–carbon composites in the literature, our material shows losses of just 22% under analogous cycling conditions.

Changes in the surface electronic states of semiconductor fine particles induced by high energy ion irradiation

Energy Technology Data Exchange (ETDEWEB)

Yamaki, Tetsuya; Asai, Keisuke; Ishigure, Kenkichi [Tokyo Univ. (Japan); Shibata, Hiromi

1997-03-01

The changes in the surface electronic states of Q-sized semiconductor particles in Langmuir-Blodgett (LB) films, induced by high energy ion irradiation, were examined by observation of ion induced emission and photoluminescence (PL). Various emission bands attributed to different defect sites in the band gap were observed at the initial irradiation stage. As the dose increased, the emissions via the trapping sites decreased in intensity while the band-edge emission developed. This suggests that the ion irradiation would remove almost all the trapping sites in the band gap. The low energy emissions, which show a multiexponential decay, were due to a donor-acceptor recombination between the deeply trapped carriers. It was found that the processes of formation, reaction, and stabilization of the trapping sites would predominantly occur under the photooxidizing conditions. (author)

High energy density in matter produced by heavy ion beams

International Nuclear Information System (INIS)

1989-07-01

This Annual Report summarizes research activities carried out in 1988 in the framework of the government-funded program 'High Energy Density in Matter produced by Heavy Ion Beams'. It addresses fundamental problems of the generation of heavy ion beams and the investigation of hot dense plasmas produced by these beams. Its initial motivation and its long-term goal is the feasibility of inertial confinement fusion by intense heavy ion beams. Two outstanding events deserve to be mentioned explicity, the Heavy Ion Inertial Fusion Conference held in Darmstadt and organized by GSI end of June and the first heavy ion beam injected into the new SIS facility in November. The former event attracted more than hundred scientists for three days to the 4th Conference in this field. This symposium showed the impressive progress since the last conference in Washington two years ago. In particular the first beams in MBE-4 at LBL and results of beam plasma interaction experiments at GSI open new directions for future investigations. The ideas for non-Lionvillean injection into storage rings presented by Carlo Rubbia will bring the discussion of driver scenarios into a new stage. The latter event is a milestone for both machine and target experiments. It characterizes the beginning of the commissioning phase for the new SIS/ESR facility which will be ready for experiments at the end of this year. The commissioning of SIS is on schedule and first experiments can start at the beginning of 1990. A status report of the accelerator project is included. Theoretical activities were continued as in previous years, many of them providing guide lines for future experiments, in particular for the radiation transport aspects and for beam-plasma interaction. (orig.)

HIGH DENSITY QCD WITH HEAVY-IONS

CERN Multimedia

The Addendum 1 to Volume 2 of the CMS Physics TDR has been published The Heavy-Ion analysis group completed the writing of a TDR summarizing the CMS plans in using heavy ion collisions to study high density QCD. The document was submitted to the LHCC in March and presented in the Open Session of the LHCC on May 9th. The study of heavy-ion physics at the LHC is promising to be very exciting. LHC will open a new energy frontier in ultra-relativistic heavy-ion physics. The collision energy of heavy nuclei at sNN = 5.5 TeV will be thirty times larger than what is presently available at RHIC. We will certainly probe quark and gluon matter at unprecedented values of energy density. The prime goal of this research programme is to study the fundamental theory of the strong interaction - Quantum Chromodynamics (QCD) - in extreme conditions of temperature, density and parton momentum fraction (low-x). Such studies, with impressive experimental and theoretical advances in recent years thanks to the wealth of high-qua...

The effect of carbon impurities on molybdenum surface morphology evolution under high-flux low-energy helium ion irradiation

International Nuclear Information System (INIS)

Tripathi, J.K.; Novakowski, T.J.; Gonderman, S.; Bharadwaj, N.; Hassanein, A.

2016-01-01

We report on the role of carbon (C) impurities, in molybdenum (Mo) fuzz evolutions on Mo surface during 100 eV He + ion irradiations. In this study we considered 0.01, 0.05, and 0.5% C + ion impurities in He + ion irradiations. For introducing such tiny C + ion impurities, gas mixtures of He and CH 4 have been chosen in following ratios; 99.95: 0.05, 99.75: 0.25, and 97.5: 2.5. Apart from these three cases, two additional cases, 100% He + ion (for Mo fuzz growth due to only He + ions) and 100% H + ion (for confirming the significance of tiny 0.04–2.0% H + ions in terms of Mo fuzz evolutions on Mo surface, if any), have also been considered. Ion energy (100 eV), ion fluence (2.6 × 10 24  ions m −2 ), and target temperature (923 K) were kept constant for each experiment and their selections were based on our previous studies [1,2]. Our study shows homogeneously populated and highly dense Mo fuzz evolutions on entire Mo surface for 100% He + ion irradiation case. Enhancement of C + ion impurities in He + ions causes a sequential reduction in Mo fuzz evolutions, leading to almost complete prevention of Mo fuzz evolutions for 0.5% C + ion impurity concentrations. Additionally, no fuzz formation for 100% H + ion irradiation at all, were seen (apart from some tiny nano-structuring, in very limited regions). This indicates that there is no significant role of H + ions in Mo fuzz evolutions (at least for such tiny amount, 0.04–2.0% H + ions). The study is significant to understand the behavior of potential high-Z plasma facing components (PFCs), in the, presence of tiny amount of C impurities, for nuclear fusion relevant applications. - Highlights: • Mo Fuzz evolutions due to low-energy high-flux 100% He + ion irradiation. • Sequential reduction in Mo fuzz evolutions with increasing C + ion impurities in He + ions. • Almost complete prevention of Mo fuzz evolutions for 0.5% C + ion impurity in He + ions. • No Mo fuzz formation for 100% H + ion

Guided transmission of highly charged ions through nanocapillaries in PET. Study of the energy dependencies

International Nuclear Information System (INIS)

Helhammer, R.; Pesic, Z.D.; Sobocinski, P.; Bundesmann, J.; Fink, D.; Stolterfoht, N.; Sulik, B.

2004-01-01

Full text: Recently we reported experiments in which slow highly charged ions are transmitted through nanocapillaries of 100nm diameter in an insulating PET foil of 10μm thickness [1]. The results of this work differ significantly from previous studies, which have been focused on capillaries in metals [2]. We measured the transmission of 3 keV Ne 7+ ions through the capillaries and focused the attention on ions whose charge has not changed during the passage through the capillary. The observation that the angular distribution for PET has a peak maximum whose position is equal to the tilt angle indicates a guiding of the Ne 7+ ion within the capillary. This guiding shows that the inner walls of the capillaries are charged up in a self-organizing process and collisions with the surface are finally prevented. We studied the time evolution of the capillary guiding as well as dependencies on the tilt angle [3]. Our most recent measurements were focussed on the investigation of the energy dependency for the guiding of Ne 7+ through capillaries. The measurements were done in an energy range from 2 keV up to 10 keV.We measured higher guiding efficiency for lower energies consistent with a previously developed model, which predicted an increase of the guiding efficiency with decreasing projectile energy [3]. In addition we found the effect of a narrower width of the angular distribution of transmitted ions. This effect is also well described by the model. However, further work is needed to explain the amount of charges to build up the deflection field at the end of the capillaries

X-ray emission in slow highly charged ion-surface collisions

International Nuclear Information System (INIS)

Watanabe, H; Abe, T; Fujita, Y; Sun, J; Takahashi, S; Tona, M; Yoshiyasu, N; Nakamura, N; Sakurai, M; Yamada, C; Ohtani, S

2007-01-01

X-rays emitted in the collisions of highly charged ions with a surface have been measured to investigate dissipation schemes of their potential energies. While 8.1% of the potential energy was dissipated in the collisions of He-like I ions with a W surface, 29.1% has been dissipated in the case of He-like Bi ions. The x-ray emissions play significant roles in the dissipation of the potential energies in the interaction of highly charged heavy ions with the surface

A high energy and power Li-ion capacitor based on a TiO2 nanobelt array anode and a graphene hydrogel cathode.

Science.gov (United States)

Wang, Huanwen; Guan, Cao; Wang, Xuefeng; Fan, Hong Jin

2015-03-25

A novel hybrid Li-ion capacitor (LIC) with high energy and power densities is constructed by combining an electrochemical double layer capacitor type cathode (graphene hydrogels) with a Li-ion battery type anode (TiO(2) nanobelt arrays). The high power source is provided by the graphene hydrogel cathode, which has a 3D porous network structure and high electrical conductivity, and the counter anode is made of free-standing TiO(2) nanobelt arrays (NBA) grown directly on Ti foil without any ancillary materials. Such a subtle designed hybrid Li-ion capacitor allows rapid electron and ion transport in the non-aqueous electrolyte. Within a voltage range of 0.0-3.8 V, a high energy of 82 Wh kg(-1) is achieved at a power density of 570 W kg(-1). Even at an 8.4 s charge/discharge rate, an energy density as high as 21 Wh kg(-1) can be retained. These results demonstrate that the TiO(2) NBA//graphene hydrogel LIC exhibits higher energy density than supercapacitors and better power density than Li-ion batteries, which makes it a promising electrochemical power source. © 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Peapod-like Li3 VO4 /N-Doped Carbon Nanowires with Pseudocapacitive Properties as Advanced Materials for High-Energy Lithium-Ion Capacitors.

Science.gov (United States)

Shen, Laifa; Lv, Haifeng; Chen, Shuangqiang; Kopold, Peter; van Aken, Peter A; Wu, Xiaojun; Maier, Joachim; Yu, Yan

2017-07-01

Lithium ion capacitors are new energy storage devices combining the complementary features of both electric double-layer capacitors and lithium ion batteries. A key limitation to this technology is the kinetic imbalance between the Faradaic insertion electrode and capacitive electrode. Here, we demonstrate that the Li 3 VO 4 with low Li-ion insertion voltage and fast kinetics can be favorably used for lithium ion capacitors. N-doped carbon-encapsulated Li 3 VO 4 nanowires are synthesized through a morphology-inheritance route, displaying a low insertion voltage between 0.2 and 1.0 V, a high reversible capacity of ≈400 mAh g -1 at 0.1 A g -1 , excellent rate capability, and long-term cycling stability. Benefiting from the small nanoparticles, low energy diffusion barrier and highly localized charge-transfer, the Li 3 VO 4 /N-doped carbon nanowires exhibit a high-rate pseudocapacitive behavior. A lithium ion capacitor device based on these Li 3 VO 4 /N-doped carbon nanowires delivers a high energy density of 136.4 Wh kg -1 at a power density of 532 W kg -1 , revealing the potential for application in high-performance and long life energy storage devices. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Ion-ion interaction and energy transfer of 4+ transuranium ions in cerium tetrafluoride

International Nuclear Information System (INIS)

Liu, G.K.; Beitz, J.V.

1990-01-01

Dynamics of excited 5f electron states of the transuranium ions Cm 4+ and Bk 4+ in CeF 4 are compared. Based on time- and wavelength-resolved laser-induced fluorescence, excitation energy transfer processes have been probed. Depending on concentration and electronic energy level structure of the studied 4+ transuranium ion, the dominant energy transfer mechanisms were identified as cross relaxation, exciton-exciton annihilation, and trapping. Energy transfer rates derived from the fitting of the observed fluorescence decays to theoretical models, based on electric multipolar ion-ion interactions, are contrasted with prior studies of 4f states of 3+ lanthanide and 3d states of transition metal ions. 16 refs., 1 tab

Experimental study of interactions of highly charged ions with atoms at keV energies. Progress report, February 16, 1993--April 15, 1994

International Nuclear Information System (INIS)

Kostroun, V.O.

1994-01-01

Experimental study of low energy, highly charged ions with other atomic species requires an advanced ion source such as an electron beam ion source, EBIS or an electron cyclotron ion source, ECRIS. Five years ago we finished the design and construction of the Cornell superconducting solenoid, cryogenic EBIS (CEBIS). Since then, this source has been in continuous operation in a program whose main purpose is the experimental study of interactions of highly charged ions with atoms at keV energies. This progress report for the period February 16, 1993 to April 15, 1994 describes the work accomplished during this time in the form of short abstracts

Study on the erosion of refractory metals in interaction with low energy ions at high temperatures of a target

International Nuclear Information System (INIS)

Vaulin, E.P.; Georgieva, N.E.; Martynenko, T.P.; Feoktistov, L.V.

1981-01-01

The experimental study on the erosion of a polycrystalline tungsten by argon ions with 50-100 eV energy in the temperature range 1000-1900 K is carried out and a theoretical analysis of sputtering rate under these conditions is given. It is shown that the sputtering rate is determined not only by ion energy but depends essentially on surface temperature. On the basis of the thermal spot'' model a semiempiric formula is obtained for dependence of sputtering coefficient on ion energy and target temperature. The estimation of cathode specific errosion in high-current discharges due to the sputtering and evaporation is performed. It is shown that depending on cathode temperature, cathode potential jump value as well as on relation of ion and electron current on a cathode the specific erosion due to individual ions shock can be higher and much higher than the specific erosion for account of evaporation [ru

Hardening of ODS ferritic steels under irradiation with high-energy heavy ions

Science.gov (United States)

Ding, Z. N.; Zhang, C. H.; Yang, Y. T.; Song, Y.; Kimura, A.; Jang, J.

2017-09-01

Influence of the nanoscale oxide particles on mechanical properties and irradiation resistance of oxide-dispersion-strengthened (ODS) ferritic steels is of critical importance for the use of the material in fuel cladding or blanket components in advanced nuclear reactors. In the present work, impact of structures of oxide dispersoids on the irradiation hardening of ODS ferritic steels was studied. Specimens of three high-Cr ODS ferritic steels containing oxide dispersoids with different number density and average size were irradiated with high-energy Ni ions at about -50 °C. The energy of the incident Ni ions was varied from 12.73 MeV to 357.86 MeV by using an energy degrader at the terminal so that a plateau of atomic displacement damage (∼0.8 dpa) was produced from the near surface to a depth of 24 μm in the specimens. A nanoindentor (in constant stiffness mode with a diamond Berkovich indenter) and a Vickers micro-hardness tester were used to measure the hardeness of the specimens. The Nix-Gao model taking account of the indentation size effect (ISE) was used to fit the hardness data. It is observed that the soft substrate effect (SSE) can be diminished substantially in the irradiated specimens due to the thick damaged regions produced by the Ni ions. A linear correlation between the nano-hardeness and the micro-hardness was found. It is observed that a higher number density of oxide dispersoids with a smaller average diameter corresponds to an increased resistance to irradiation hardening, which can be ascribed to the increased sink strength of oxides/matrix interfaces to point defects. The rate equation approach and the conventional hardening model were used to analyze the influence of defect clusters on irradiation hardening in ODS ferritic steels. The numerical estimates show that the hardening caused by the interstitial type dislocation loops follows a similar trend with the experiment data.

[Search for strange quark matter and antimatter produced in high energy heavy ion collisions

International Nuclear Information System (INIS)

1992-01-01

This document describes the development and progress of our group's research program in high energy heavy ion physics. We are a subset of the Yale experimental high energy physics effort (YAUG group) who became interested in the physics of high energy heavy ions in 1988. Our interest began with the possibility of performing significant searches for strange quark matter. As we learned more about the subject and as we gained experimental experience through our participation in AGS experiment 814, our interests have broadened. Our program has focused on the study of new particles, including (but not exclusively) strange quark matter, and the high sensitivity measurement of other composite nuclear systems such as antinuclei and various light nuclei. The importance of measurements of the known, but rare, nuclear systems lies in the study of production mechanisms. A good understanding of the physics and phenomenology of rare composite particle production in essential for the interpretation of limits to strange quark matter searches. We believe that such studies will also be useful in probing the mechanisms involved in the collision process itself. We have been involved in the running and data analysis for AGS E814. We have also worked on the R ampersand D for AGS E864, which is an approved experiment designed to reach sensitivities where there will be a good chance of discovering strangelets or of setting significant limits on the parameters of strange quark matter

Multi-megajoule heating of large tokamaks with high energy heavy ion beams

International Nuclear Information System (INIS)

Dei-Cas, R.

1981-07-01

The fast neutral injection heating and RF heating for tokamak like plasmas are now well established. We consider in this paper the use of high energy (approximately 1 GeV) heavy ions (Xe 132 ) to reach ignition in JET or INTOR like tokamaks. The main advantages of such a method will be outlined. The capture and the confinement of heavy ions have been analysed in a particular case and with the described RF linac it seems possible to inject in the order of 50 MJ in 1 sec with a modest increase of the effective charge Zsub(eff)<1.05 in a JET-like plasma for a particle life time of 1 sec and then the additional radiated power should be maintained at a relatively low level in comparison to the injected power

Measurements of Ion Stopping around the Bragg Peak in High-Energy-Density Plasmas

Science.gov (United States)

Frenje, Johan

2015-11-01

Over the last few decades, ion stopping in weakly- to strongly-coupled High-Energy-Density (HED) plasmas has been subject to extensive analytical and numerical studies, but only a limited set of experimental data exists to check the validity of these theories. Most of these experiments also did not probe the detailed characteristics of the Bragg peak (peak ion stopping) where the ion velocity is similar to the average thermal electron velocity. To the best of our knowledge, only one exploratory attempt to do this was conducted by Hicks et al., who were able to describe qualitatively the behavior of the Bragg peak for one plasma condition. The work described in this presentation makes significant advances over previous experimental efforts by quantitatively assessing the characteristics of the ion stopping, ranging from low-velocity stopping, through the Bragg peak, to high-velocity stopping for different HED plasma conditions. This was achieved by measuring the energy loss of DD-tritons, D3He-alphas, DD-protons and D3He-protons, with distinctly different velocities, and the results indicate that the stopping power varies strongly with Te and ne. This effort represents the first experimental test of state-of-art plasma-stopping-power theories around the Bragg peak, which is an important first step in our efforts of getting a fundamental understanding of DT-alpha stopping in HED plasmas, a prerequisite for understanding ignition margins in various implosion designs with varying hot spot areal density at the National Ignition Facility. The work described here was performed in part at the LLE National Laser User's Facility (NLUF), and was supported in part by US DOE (Grant No. DE-FG03- 03SF22691), LLNL (subcontract Grant No. B504974) and LLE (subcontract Grant No. 412160-001G).

High-Phosphorus, Low-Calcium Dietary Intakes and Bone Effects of Physical Training

National Research Council Canada - National Science Library

Zerath, Erik

2003-01-01

.... Diet inquiries showed changes in calcium and phosphorus intakes. This study is aimed at investigating the effects of physical activity on bone tissue in the context of high-phosphorus and low-calcium intakes. Sedentary (SED) and trained (TR...

Preparation of highly dispersed palladium–phosphorus nanoparticles and its electrocatalytic performance for formic acid electrooxidation

International Nuclear Information System (INIS)

Sun Hanjun; Xu Jiangfeng; Fu Gengtao; Mao Xinbiao; Zhang, Lu; Chen Yu; Zhou Yiming; Lu Tianhong; Tang Yawen

2012-01-01

Highly dispersed and ultrafine palladium–phosphorus (Pd–P) nanoparticles (NPs) are prepared with a novel phosphorus reduction method. The structural and electronic properties of Pd–P NPs are characterized using Fourier transform infrared (FT-IR), energy dispersive spectrometer (EDS), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS) and transmission electron microscopy (TEM). The electrooxidation of formic acid on Pd–P NPs are investigated by using cyclic voltammetry, chronoamperometry and CO-stripping measurements. The physical characterizations indicate the doped P element can enhance the content of Pd 0 species in Pd NPs, decrease the particle size and improve the dispersion of Pd–P NPs. The electrochemical measurements show the Pd–P NPs have a better catalytic performance for formic acid electrooxidation than Pd NPs.

Mechanism of long-range penetration of low-energy ions in botanic samples

International Nuclear Information System (INIS)

Liu Feng; Wang Yugang; Xue Jianming; Wang Sixue; Du Guanghua; Yan Sha; Zhao Weijiang

2002-01-01

The authors present experimental evidence to reveal the mechanism of long-range penetration of low-energy ions in botanic samples. In the 100 keV Ar + ion transmission measurement, the result confirmed that low-energy ions could penetrate at least 60 μm thick kidney bean slices with the probability of about 1.0 x 10 -5 . The energy spectrum of 1 MeV He + ions penetrating botanic samples has shown that there is a peak of the count of ions with little energy loss. The probability of the low-energy ions penetrating the botanic sample is almost the same as that of the high-energy ions penetrating the same samples with little energy loss. The results indicate that there are some micro-regions with mass thickness less than the projectile range of low-energy ions in the botanic samples and they result in the long-range penetration of low-energy ions in botanic samples

Critical issues in the formation of quantum computer test structures by ion implantation

Energy Technology Data Exchange (ETDEWEB)

Schenkel, T.; Lo, C. C.; Weis, C. D.; Schuh, A.; Persaud, A.; Bokor, J.

2009-04-06

The formation of quantum computer test structures in silicon by ion implantation enables the characterization of spin readout mechanisms with ensembles of dopant atoms and the development of single atom devices. We briefly review recent results in the characterization of spin dependent transport and single ion doping and then discuss the diffusion and segregation behaviour of phosphorus, antimony and bismuth ions from low fluence, low energy implantations as characterized through depth profiling by secondary ion mass spectrometry (SIMS). Both phosphorus and bismuth are found to segregate to the SiO2/Si interface during activation anneals, while antimony diffusion is found to be minimal. An effect of the ion charge state on the range of antimony ions, 121Sb25+, in SiO2/Si is also discussed.

Atomic physics of highly charged ions in an electron beam ion trap

International Nuclear Information System (INIS)

Marrs, R.E.

1990-07-01

Two electron beam ion traps are in use at LLNL for the purpose of studying the properties of very highly charged ions and their interactions with electrons. This paper reviews the operation of the traps and discusses recent experiments in three areas: precision transition energy measurements in the limit of very high ion charge, dielectronic recombination measurements for the He-like isoelectronic sequence, and measurements of x-ray polarization. 22 refs., 11 figs., 1 tab

Material-related issues at high-power and high-energy ion beam facilities

CERN Document Server

Bender, M.; Tomut, M.; Trautmann, C.

2015-01-01

When solids are exposed to energetic ions (MeV-GeV), their physical and chemical structure can be severely modified. The change is governed by ultrafast dynamical processes starting from the deposition of large energy densities, electronic excitation and ionization processes, and finally damage creation in the atomic lattice system. In many materials, each projectile creates a cylindrical track with a few nanometers in diameter and up to many μm in length. To study and monitor the creation of damage, the GSI irradiation facility dedicated to materials science provides different in-situ and on-line techniques such as high resolution microscopy, X-ray diffraction, optical absorption spectroscopy, thermal imaging and residual gas analysis. The irradiation experiments can be performed under various gas atmospheres and under cryogenic or elevated temperature.

Study of phosphorus implanted and annealed silicon by electrical measurements and ion channeling technique

CERN Document Server

Hadjersi, T; Zilabdi, M; Benazzouz, C

2002-01-01

We investigated the effect of annealing temperature on the electrical activation of phosphorus implanted into silicon. The measurements performed using spreading resistance, four-point probe and ion channeling techniques have allowed us to establish the existence of two domains of variation of the electrical activation (350-700 deg. C) and (800-1100 deg. C). The presence of reverse annealing and the annihilation of defects have been put in a prominent position in the first temperature range. It has been shown that in order to achieve a complete electrical activation, the annealing temperature must belong to the second domain (800-1100 deg. C).

Highly charged ion trapping and cooling

International Nuclear Information System (INIS)

Beck, B. R.; Church, D. A.; Gruber, L.; Holder, J. P.; Schneider, D.; Steiger, J.

1998-01-01

In the past few years a cryogenic Penning trap (RETRAP) has been operational at the Electron Beam Ion Trap (EBIT) facility at Lawrence Livermore National Laboratory. The combination of RETRAP and EBIT provides a unique possibility of producing and re-trapping highly charged ions and cooling them to very low temperatures. Due to the high Coulomb potentials in such an ensemble of cold highly charged ions the Coulomb coupling parameter (the ratio of Coulomb potential to the thermal energy) can easily reach values of 172 and more. To study such systems is not only of interest in astrophysics to simulate White Dwarf star interiors but opens up new possibilities in a variety of areas (e.g. laser spectroscopy), cold highly charged ion beams

The low-energy-beam and ion-trap facility at NSCL/MSU

Energy Technology Data Exchange (ETDEWEB)

Schwarz, S. E-mail: schwarz@nscl.msu.edu; Bollen, G.; Lawton, D.; Lofy, P.; Morrissey, D.J.; Ottarson, J.; Ringle, R.; Schury, P.; Sun, T.; Varentsov, V.; Weissman, L

2003-05-01

The goal of the low-energy-beam and ion-trap (LEBIT) project is to convert the high-energy exotic beams produced at NSCL/MSU into low-energy low-emittance beams. This beam manipulation will be done by a combination of a high-pressure gas stopping cell and a radio-frequency quadrupole ion accumulator and buncher. The first experimental program to profit from the low-energy beams produced will be high-accuracy mass measurements on very short-lived isotopes with a 9.4 T Penning trap system. The status of the project is presented with an emphasis on recent stopping tests range of 100 MeV/A {sup 40}Ar{sup 18+} ions in a gas cell.

The low-energy-beam and ion-trap facility at NSCL/MSU

International Nuclear Information System (INIS)

Schwarz, S.; Bollen, G.; Lawton, D.; Lofy, P.; Morrissey, D.J.; Ottarson, J.; Ringle, R.; Schury, P.; Sun, T.; Varentsov, V.; Weissman, L.

2003-01-01

The goal of the low-energy-beam and ion-trap (LEBIT) project is to convert the high-energy exotic beams produced at NSCL/MSU into low-energy low-emittance beams. This beam manipulation will be done by a combination of a high-pressure gas stopping cell and a radio-frequency quadrupole ion accumulator and buncher. The first experimental program to profit from the low-energy beams produced will be high-accuracy mass measurements on very short-lived isotopes with a 9.4 T Penning trap system. The status of the project is presented with an emphasis on recent stopping tests range of 100 MeV/A 40 Ar 18+ ions in a gas cell

Fabrication and demonstration of high energy density lithium ion microbatteries

Science.gov (United States)

Sun, Ke

Since their commercialization by Sony two decades ago, Li-ion batteries have only experienced mild improvement in energy and power performance, which remains one of the main hurdles for their widespread implementation in applications outside of powering compact portable devices, such as in electric vehicles. Li-ion batteries must be advanced through a disruptive technological development or a series of incremental improvements in chemistry and design in order to be competitive enough for advanced applications. As it will be introduced in this work, achieving this goal by new chemistries and chemical modifications does not seem to be promising in the short term, so efforts to fully optimize existing systems must be pursued at in parallel. This optimization must be mainly relying on the modification and optimizations of micro and macro structures of current battery systems. This kind of battery architecture study will be even more important when small energy storage devices are desired to power miniaturized and autonomous gadgets, such as MEMs, micro-robots, biomedical sensors, etc. In this regime, the limited space available makes requirements on electrode architecture more stringent and the assembly process more challenging. Therefore, the study of battery assembly strategies for Li-ion microbatteries will benefit not only micro-devices but also the development of more powerful and energetic large scale battery systems based on available chemistries. In chapter 2, preliminary research related to the mechanism for the improved rate capability of cathodes by amorphous lithium phosphate surficial films will be used to motivate the potential for structural optimization of existing commercial lithium ion battery electrode. In the following chapters, novel battery assembly techniques will be explored to achieve new battery architectures. In chapter 3, direct ink writing will be used to fabricate 3D interdigitated microbattery structures that have superior areal energy

Light ion beam approach to ICF ignition, gain, and energy production

International Nuclear Information System (INIS)

Olson, R.; Allshouse, G.; Cook, D.

1993-01-01

The US Department of Energy is supporting research oriented toward both near-term defense applications as well as long-term energy applications of inertial confinement fusion (ICF). The ICF programs at Sandia National Laboratories (SNL) is directed toward validating light ions as an efficient driver for these applications. The light ion laboratory microfusion facility (LMF) is envisioned as a facility in which high gain ICF targets could be developed and utilized in defense-related experiments. The LIBRA light ion beam commercial reactor study provides a baseline approach towards the use of the high gain light ion ICF technology as a source of commercial electrical energy

Light ion beam approach to ICF ignition, gain, and energy production

International Nuclear Information System (INIS)

Olson, R.; Allshouse, G.; Cook, D.

1994-01-01

The U.S. Department of Energy is supporting research oriented toward both near-term defense applications as well as long-term energy applications of inertial confinement fusion (ICF). The ICF program at Sandia National Laboratories (SNL) is directed toward validating light ions as an efficient driver for these applications. The light ion laboratory microfusion facility (LMF) is envisioned as a facility in which high gain ICF targets could be developed and utilized in defense-related experiments. The LIBRA light ion beam commercial reactor study provides a baseline approach towards the use of the high gain light ion ICF technology as a source of commercial electrical energy. (author)

Radiation stability of nanocrystalline ZrN coatings irradiated with high energy Xe and Bi ions

International Nuclear Information System (INIS)

Skuratov, V.A.; Sokhatsky, A.S.; Uglov, V.V.; Zlotski, S.V.; Van Vuuren, A.J.; Neethling, Jan; O'Connell, J.

2011-01-01

Swift Xe and Bi ion irradiation effects in nanocrystalline ZrN coatings as a function of ion fluence are reported. Zirconium nitride films of different thickness (0.1, 3, 10 and 20 micrometers) synthesized by vacuum arc-vapour deposition in nanocrystalline state (average size of crystallites is ∼4 nm) were irradiated with 167 MeV Xe and 695 MeV Bi ions to fluences in the range 3x10 12 ÷2.6x10 15 cm -2 (Xe) and 10 12 x10 13 cm -2 (Bi) and studied using XRD and TEM techniques. No evidence of amorphization due to high level ionizing energy losses has been found. The measurements of lattice parameter have revealed nonmonotonic dependence of the stress level in irradiated samples on ion fluence. (authors)

p-type ZnO films with solid-source phosphorus doping by molecular-beam epitaxy

International Nuclear Information System (INIS)

Xiu, F.X.; Yang, Z.; Mandalapu, L.J.; Liu, J.L.; Beyermann, W. P.

2006-01-01

Phosphorus-doped p-type ZnO films were grown on r-plane sapphire substrates using molecular-beam epitaxy with a solid-source GaP effusion cell. X-ray diffraction spectra and reflection high-energy electron diffraction patterns indicate that high-quality single crystalline (1120) ZnO films were obtained. Hall and resistivity measurements show that the phosphorus-doped ZnO films have high hole concentrations and low resistivities at room temperature. Photoluminescence (PL) measurements at 8 K reveal a dominant acceptor-bound exciton emission with an energy of 3.317 eV. The acceptor energy level of the phosphorus dopant is estimated to be 0.18 eV above the valence band from PL spectra, which is also consistent with the temperature dependence of PL measurements

CR-39 nuclear track detector application for the diagnostics of low energy high power ion beams

Energy Technology Data Exchange (ETDEWEB)

Opekounov, M S; Pechenkin, S A; Remnev, G E [Nuclear Physics Institute, Tomsk (Russian Federation); Ivonin, I V [Siberian Physical-Technical Institute, Tomsk (Russian Federation)

1997-12-31

The results of investigation of the spectral composition of ion beams generated by the magneto-insulated ion diode of the MUK-M and TEMP accelerators. The energy and mass characteristics of the accelerated ion beam were determined by a Thomson spectrometer with a CR-39 plate detector (MOM - Atomki Nuclear Track Detector, Type MA-ND/p). The accelerated ion energy was from 40 to 240 keV. The ion current density range was from 1 to 10 A/cm{sup 2}. The mass composition contained hydrogen, nitrogen, carbon and aluminum ions. The individual track analysis showed the track form, depth and diameter in dependence on the ion mass and energy. (author). 2 figs., 5 refs.

High energy (MeV) ion beam modifications of sputtered MoS2 coatings on sapphire

International Nuclear Information System (INIS)

Bhattacharya, R.S.; Rai, A.K.; Erdemir, A.

1991-01-01

The present article reports on the results of our investigations of high-energy (MeV) ion irradiation on the microstructural and tribological properties of dc magnetron sputtered MoS 2 films. Films of thicknesses 500-7500 A were deposited on NaCl, Si and sapphire substrates and subsequently ion irradiated by 2 MeV Ag + ions at a dose of 5x10 15 cm -2 . Scanning and transmission electron microscopy. Rutherford backscattering and X-ray diffraction techniques were utilized to study the structural, morphological and compositional changes of the film due to ion irradiation. The friction coefficient and sliding life were determined by pin-on-disc tests. Both as-deposited and ion-irradiated films were found to be amorphous having a stoichiometry of MoS 1.8 . A low friction coefficient in the range 0.03-0.04 was measured for both as-deposited and ion-irradiated films. However, the sliding life of ion-irradiated film was found to increase more than tenfold compared to as-deposited films indicating improved bonding at the interface. (orig.)

The effect of carbon impurities on molybdenum surface morphology evolution under high-flux low-energy helium ion irradiation

Energy Technology Data Exchange (ETDEWEB)

Tripathi, J.K., E-mail: jtripat@purdue.edu; Novakowski, T.J.; Gonderman, S.; Bharadwaj, N.; Hassanein, A.

2016-09-15

We report on the role of carbon (C) impurities, in molybdenum (Mo) fuzz evolutions on Mo surface during 100 eV He{sup +} ion irradiations. In this study we considered 0.01, 0.05, and 0.5% C{sup +} ion impurities in He{sup +} ion irradiations. For introducing such tiny C{sup +} ion impurities, gas mixtures of He and CH{sub 4} have been chosen in following ratios; 99.95: 0.05, 99.75: 0.25, and 97.5: 2.5. Apart from these three cases, two additional cases, 100% He{sup +} ion (for Mo fuzz growth due to only He{sup +} ions) and 100% H{sup +} ion (for confirming the significance of tiny 0.04–2.0% H{sup +} ions in terms of Mo fuzz evolutions on Mo surface, if any), have also been considered. Ion energy (100 eV), ion fluence (2.6 × 10{sup 24} ions m{sup −2}), and target temperature (923 K) were kept constant for each experiment and their selections were based on our previous studies [1,2]. Our study shows homogeneously populated and highly dense Mo fuzz evolutions on entire Mo surface for 100% He{sup +} ion irradiation case. Enhancement of C{sup +} ion impurities in He{sup +} ions causes a sequential reduction in Mo fuzz evolutions, leading to almost complete prevention of Mo fuzz evolutions for 0.5% C{sup +} ion impurity concentrations. Additionally, no fuzz formation for 100% H{sup +} ion irradiation at all, were seen (apart from some tiny nano-structuring, in very limited regions). This indicates that there is no significant role of H{sup +} ions in Mo fuzz evolutions (at least for such tiny amount, 0.04–2.0% H{sup +} ions). The study is significant to understand the behavior of potential high-Z plasma facing components (PFCs), in the, presence of tiny amount of C impurities, for nuclear fusion relevant applications. - Highlights: • Mo Fuzz evolutions due to low-energy high-flux 100% He{sup +} ion irradiation. • Sequential reduction in Mo fuzz evolutions with increasing C{sup +} ion impurities in He{sup +} ions. • Almost complete prevention of Mo

Achieving high baryon densities in the fragmentation regions in heavy ion collisions at top RHIC energy

International Nuclear Information System (INIS)

Li, Ming; Kapusta, Joseph I.

2017-01-01

Heavy ion collisions at extremely high energy, such as the top energy at RHIC, exhibit the property of transparency where there is a clear separation between the almost net-baryon-free central rapidity region and the net-baryon-rich fragmentation region. We calculate the net-baryon rapidity loss and the nuclear excitation energy using the energy-momentum tensor obtained from the McLerran-Venugopalan model. Nuclear compression during the collision is further estimated using a simple space-time picture. The results show that extremely high baryon densities, about twenty times larger than the normal nuclear density, can be achieved in the fragmentation regions. (paper)

High-resolution X-ray spectra from low-temperature, highly charged ions

International Nuclear Information System (INIS)

Beiersdorfer, P.

1996-09-01

The electron beam ion traps (EBIT) at Livermore were designed for studying the x-ray emission of highly charged ions produced and excited by a monoenergetic electron beam. The precision with which the x-ray emission can be analyzed has recently been increased markedly when it became possible to decouple the temperature of the ions from the energy of the electron beam by several orders of magnitude. By adjusting the trap parameters, ion temperatures as low as 15.8±4.4 eV for Ti 20+ and 59.4±9.9 eV for Cs 45+ were achieved. These temperatures were more than two orders of magnitude lower than the energy of the multi-keV electron beam used for the production and excitation of the ions. A discussion of the techniques used to produce and study low-temperature highly charged ions is presented in this progress report. The low ion temperatures enabled measurements heretofore impossible. As an example, a direct observation of the natural line width of fast electric dipole allowed x-ray transitions is described. From the observed natural line width and b making use of the time-energy relations of the uncertainty principle we were able to determine a radiative transition rate of 1.65 fs for the 2p-3d resonance transition in neonlike Cs 45+ . A brief discussion of other high-precision measurements enabled by our new technique is also given

Multiple relaxation processes in high-energy ion irradiated kapton-H polyimide: Thermally stimulated depolarization current study

International Nuclear Information System (INIS)

Garg, Maneesha; Quamara, J.K.

2006-01-01

High-energy ion irradiation effects on the thermally stimulated depolarization current (Tdc) behaviour of kapton-H samples (12.5 μm) irradiated with 50 MeV Li ion (fluence 5 x 10 4 , 10 5 and 5 x 10 5 ions/cm 2 ) have been investigated. The TSDC spectra of the irradiated samples reveal that the β-peak (appearing around 80-110 deg. C) associated with dipolar relaxation has been significantly affected owing to the demerization of carbonyl groups due to irradiation. The TSDC spectra also reveal a new relaxation process (termed as γ-relaxation) around 30 deg. C, due to increased water absorptivity in irradiated samples. The peak around 200 deg. C (α-peak) associated with space charge relaxation process also shows a behavioural change with ion irradiation. The peak not only shifts towards the higher temperature with increasing fluence but also show an increase in its activation energy (0.33-0.99 eV) with increasing polarizing field. The creation of new deep energy trap centers due to the formation of conjugated bonds after irradiation is responsible for this modification. The Cole-Cole distribution curves show the formation of new sub-polar group with different characteristic relaxation time

Studies on the production of high energy densities in matter by intense heavy-ion beams

International Nuclear Information System (INIS)

Jacoby, J.

1989-08-01

In the framework of the present thesis the interaction of an intense heavy-ion beam with a small, but macroscopical amount of matter is studied. Thereby high energy densities in the target matter are produced. For this experiment it was for the first time possible to heat matter with ion beams from conventional heavy-ion accelerators up to plasma conditions. A KR + -ion beam was first accelerated with the heavy-ion accelerator MAXILAC to 45 keV/u and then focussed by a fine-focusing lens to a closed xenon gas target. The light emitted from the target was space- and time resolved taken up by a spectrometer as well as by a streak and CCD camera. Thereby the radial development of the plasma and the penetration behaviour of the ion beam was observed. The free electron density of the plasma was determined from the Stark broadening of emission lines (n e ≅ 4x10 16 cm -3 ). The temperature could be determined by different methods (shock-wave velocity, degree of ionization, line ratios). The electron temperature amounted in the center of the pipe to kT ≅ 0.75 eV. For the opacity of the target by which the emitted light power is determined under the assumption of the two-dimensional model (equilibrium between emitted and absorbed energy) the value κ p ≅ 7700 cm 2 /g resulted. (orig./HSI) [de

High energy P implants in silicon

International Nuclear Information System (INIS)

Raineri, V.; Cacciato, A.; Benyaich, F.; Priolo, F.; Rimini, E.; Galvagno, G.; Capizzi, S.

1992-01-01

Phosphorus ions in the energy range 0.25-1 MeV and in the dose range 2x10 13 -1x10 15 P/cm 2 were implanted into (100) Si single crystal at different tilt angles. In particular channeling and random conditions were investigated. For comparison some implants were performed on samples with a 2 μm thick surface amorphous layer. Chemical concentration P profiles were obtained by secondary ion mass spectrometry. Carrier concentration and mobility profile measurements were carried out by sheet resistance and Hall measurements on implanted van der Pauw patterns. Carrier concentration profiles were also obtained by spreading resistance (SR) measurements. The damage in the as-implanted samples was determined by backscattering and channeling spectrometry (RBS) as a function of the dose and implantation energy. Comparison of random implants in crystal with implants in amorphous layers shows that in the first case it is impossible to completely avoid the channeling tail. In the implants performed under channeling conditions at low doses the P profiles are flat over more than 2 μm thick layers. Furthermore, by increasing the implanted dose, the shape of the profiles dramatically changes due to the dechanneling caused by the crystal disorder. The data are discussed and compared with Monte Carlo simulations using the MARLOWE code. A simple description of the electronic energy loss provides an excellent agreement between the calculated and experimental profiles. (orig.)

Nuclear structure studies with low-energy light ions: fundamental and applied

International Nuclear Information System (INIS)

Mazumdar, I.

2016-01-01

Studies in low and medium energy nuclear physics have been dominated by heavy-ion induced reactions for last five decades. Heavy-ion induced nuclear reactions have enriched our knowledge of the structural evolutions and intricacies of reaction dynamics of the nuclear many-body systems. However, the emergence and rise of heavy-ion physics have seen a general decline in studies with low- and medium-energy light-ion beams. The harsh reality of dwindling number of low-energy light ion facilities adversely affect research in nuclear physics. Very low-energy and high current light-ion facilities immediately conjures up in our minds the studies in nuclear astrophysics. Measurements of light-ion capture cross sections and astrophysical S factors are the major themes of research at most of the light-ion facilities. However, the importance low energy light-ion beams is multifarious. A variety of measurements providing vital support and inputs to heavy-ion research can only be carried out at the low-energy, light-ion facilities. Light-ion beams are also useful for generation of mono-energetic neutron beams. In this talk I will draw from some of our recent measurements to show the importance of light-ion beams in nuclear astrophysics and also in applied nuclear physics. (author)

The low-energy-beam and ion-trap facility at NSCL/MSU

CERN Document Server

Schwarz, S; Lawton, D; Lofy, P; Morrissey, D J; Ottarson, J; Ringle, R; Schury, P; Sun, T; Varentsov, V; Weissman, L

2003-01-01

The goal of the low-energy-beam and ion-trap (LEBIT) project is to convert the high-energy exotic beams produced at NSCL/MSU into low-energy low-emittance beams. This beam manipulation will be done by a combination of a high-pressure gas stopping cell and a radio-frequency quadrupole ion accumulator and buncher. The first experimental program to profit from the low-energy beams produced will be high-accuracy mass measurements on very short-lived isotopes with a 9.4 T Penning trap system. The status of the project is presented with an emphasis on recent stopping tests range of 100 MeV/A sup 4 sup 0 Ar sup 1 sup 8 sup + ions in a gas cell.

LEBIT - a low-energy beam and ion trap facility at NSCL/MSU

International Nuclear Information System (INIS)

Schwarz, S.; Bollen, G.; Davies, D.; Lawton, D.; Lofy, P.; Morrissey, D. J.; Ottarson, J.; Ringle, R.; Schury, P.; Sun, T.; VanWasshenova, D.; Sun, T.; Weissman, L.; Wiggins, D.

2003-01-01

The Low Energy Beam and Ion Trap (LEBIT) Project aims to convert the high-energy exotic beams produced at NSCL/MSU into low-energy low-emittance beams. A combination of a high-pressure gas stopping cell and a radiofrequency quadrupole (RFQ) ion accumulator and buncher will be used to manipulate the beam accordingly. High-accuracy mass measurements on very short-lived isotopes with a 9.4 T Penning trap system will be the first experimental program to profit from the low-energy beams. The status of the project is presented with a focus on recent stopping tests of 100-140 MeV/A Ar18+ ions in a gas cell

High energy radiation fluences in the ISS-USLab: Ion discrimination and particle abundances

International Nuclear Information System (INIS)

Zaconte, Veronica; Casolino, Marco; Di Fino, Luca; La Tessa, Chiara; Larosa, Marianna; Narici, Livio; Picozza, Piergiorgio

2010-01-01

The ALTEA (Anomalous Long Term Effects on Astronauts) detector was used to characterize the radiation environment inside the USLab of the International Space Station (ISS), where it measured the abundances of ions from Be to Fe. We compare the ALTEA results with Alteino results obtained in the PIRS module of the Russian segment of the ISS, and normalize to the high energy Si abundances given by Simpson. These are the first particle spectral measurements, which include ions up to Fe, performed in the USLab. The small differences observed between those made inside the USLab and the Simpson abundances can be attributed to the transport through the spacecraft hull. However, the low abundance of Fe cannot be attributed to only this process.

Damage growth in Si during self-ion irradiation: A study of ion effects over an extended energy range

International Nuclear Information System (INIS)

Holland, O.W.; El-Ghor, M.K.; White, C.W.

1989-01-01

Damage nucleation/growth in single-crystal Si during ion irradiation is discussed. For MeV ions, the rate of growth as well as the damage morphology are shown to vary widely along the track of the ion. This is attributed to a change in the dominant, defect-related reactions as the ion penetrates the crystal. The nature of these reactions were elucidated by studying the interaction of MeV ions with different types of defects. The defects were introduced into the Si crystal prior to high-energy irradiation by self-ion implantation at a medium energy (100 keV). Varied damage morphologies were produced by implanting different ion fluences. Electron microscopy and ion-channeling measurements, in conjunction with annealing studies, were used to characterize the damage. Subtle changes in the predamage morphology are shown to result in markedly different responses to the high-energy irradiation, ranging from complete annealing of the damage to rapid growth. These divergent responses occur over a narrow range of dose (2--3 times 10 14 cm -2 ) of the medium-energy ions; this range also marks a transition in the growth behavior of the damage during the predamage implantation. A model is proposed which accounts for these observations and provides insight into ion-induced growth of amorphous layers in Si and the role of the amorphous/crystalline interface in this process. 15 refs, 9 figs

An energy-filtering device coupled to a quadrupole mass spectrometer for soft-landing molecular ions on surfaces with controlled energy

Energy Technology Data Exchange (ETDEWEB)

Bodin, A.; Laloo, R.; Abeilhou, P.; Guiraud, L.; Gauthier, S.; Martrou, D. [Nanosciences Group, CEMES, CNRS UPR 8011 and University Toulouse III - Paul Sabatier, 29 rue Jeanne Marvig, BP94347, F-31055 Toulouse Cedex 4 (France)

2013-09-15

We have developed an energy-filtering device coupled to a quadrupole mass spectrometer to deposit ionized molecules on surfaces with controlled energy in ultra high vacuum environment. Extensive numerical simulations as well as direct measurements show that the ion beam flying out of a quadrupole exhibits a high-energy tail decreasing slowly up to several hundred eV. This energy distribution renders impossible any direct soft-landing deposition of molecular ions. To remove this high-energy tail by energy filtering, a 127° electrostatic sector and a specific triplet lenses were designed and added after the last quadrupole of a triple quadrupole mass spectrometer. The results obtained with this energy-filtering device show clearly the elimination of the high-energy tail. The ion beam that impinges on the sample surface satisfies now the soft-landing criterion for molecular ions, opening new research opportunities in the numerous scientific domains involving charges adsorbed on insulating surfaces.

Determination of organic phosphorus in UO2C2O4·TRPO complex

International Nuclear Information System (INIS)

Guo Yifei; Yuan Jianhua; Liang Junfu; Jiao Rongzhou; Liu Xiuqin

2001-01-01

Organic phosphorus in UO 2 C 2 O 4 ·TRPO complex is converted to inorganic phosphorous with H 2 SO 4 -HNO 3 -H 2 O 2 wet cinefaction method. In 0.14 mol/L H 2 SO 4 solution containing water soluble poly vinylalcohol as stabilizing agent, the highly sensitive ion-associates are formed by the reaction of basic dye ethyl violet with heteropoly molybdophosphoric blue. Spectrophotometric method is used for determination of phosphorus with these ion-associates. The absorbance maximum is at 620 nm. Determination of phosphorus is not affected with mass ratios R(UO 2 2+ /P) ≤ 1.4 x 10 3 , R(C 2 O 4 2- /P) ≤ 8.8 x 10 2 and R(C 2 O 4 2- /P ≤ 3.6 x 10 4 (one time wet cinefaction must be carried out). In aqueous phase, phosphorus can be directly developed and determined. This method is contrasted with poly vinylalcohol-Rodamine B-heteropoly molybdophosphoric blue, analytical results are in good coincidence. Conversion ratio of phosphorus is 99.8% - 101.1%. The minimum detection limit is 0.02 mg/L. The relative standard deviation is 3%. The recovery ratio is 97% - 103%

High energy ion irradiation effects on polymer materials. LET dependence of G value of scission of polymethylmethacrylate (PMMA)

Energy Technology Data Exchange (ETDEWEB)

Kudoh, H; Sasuga, T; Seguchi, T [Japan Atomic Energy Research Inst., Takasaki, Gunma (Japan). Takasaki Radiation Chemistry Research Establishment

1997-03-01

Linear energy transfer (LET) dependence on the probability of main chain scission of polymethylmethacrylate (PMMA) was investigated. The probability was obtained from decreases in molecular weight measured by the gel permeation chromatography (GPC), and LET was evaluated by TRIM code. The scission probability as a function of LET was almost constant in the low LET, and decreased in the high LET ion irradiation. The mechanism was interpreted from the model of spur-overlapping along an ion`s path. (author)

Studies on the production of high energy density in matter with intense heavy-ion beams

International Nuclear Information System (INIS)

Jacoby, J.

1989-01-01

In the framework of the present thesis the interaction of an intense heavy-ion beam with a small, but macroscopic, amount of matter is studied. Thereby high energy densities are produced in the target matter. For this experiment it was for the first time possible to heat matter with ion beams from conventional heavy-ion accelerators up to plasma conditions. A Kr + ion beam was first accelerated with the heavy-ion accelerator MAXILAC to 45 keV/u and then focused by a fine-focusing lens on a closed xenon gas target. The light emitted from the target was space- and time-resolved taken up with a spectrometer as well a streak and CCD camera. Thereby the radial development of the plasma and the penetration behaviour of the ion beam were consecuted. The free-electron density of the plasma was determined from the Stark-broadening of emission lines (n e ≅ 4x10 16 cm -3 ). The electron temperature amounted in the center of the pipelet kT ≅ 0.75 eV. (orig./HSI) [de

Homologous recombination contributes to the repair of DNA double-strand breaks induced by high-energy iron ions

Energy Technology Data Exchange (ETDEWEB)

Zafar, Faria; Seidler, Sara B.; Kronenberg, Amy; Schild, David; Wiese, Claudia

2010-06-29

To test the contribution of homologous recombinational repair (HRR) in repairing DNA damaged sites induced by high-energy iron ions, we used: (1) HRR-deficient rodent cells carrying a deletion in the RAD51D gene and (2) syngeneic human cells impaired for HRR by RAD51D or RAD51 knockdown using RNA interference. We show that in response to iron ions, HRR contributes to cell survival in rodent cells, and that HRR-deficiency abrogates RAD51 foci formation. Complementation of the HRR defect by human RAD51D rescues both enhanced cytotoxicity and RAD51 foci formation. For human cells irradiated with iron ions, cell survival is decreased, and, in p53 mutant cells, the levels of mutagenesis are increased when HRR is impaired. Human cells synchronized in S phase exhibit more pronounced resistance to iron ions as compared with cells in G1 phase, and this increase in radioresistance is diminished by RAD51 knockdown. These results implicate a role for RAD51-mediated DNA repair (i.e. HRR) in removing a fraction of clustered lesions induced by charged particle irradiation. Our results are the first to directly show the requirement for an intact HRR pathway in human cells in ensuring DNA repair and cell survival in response to high-energy high LET radiation.

Homologous recombination contributes to the repair of DNA double-strand breaks induced by high-energy iron ions

International Nuclear Information System (INIS)

Zafar, Faria; Seidler, Sara B.; Kronenberg, Amy; Schild, David; Wiese, Claudia

2010-01-01

To test the contribution of homologous recombinational repair (HRR) in repairing DNA damaged sites induced by high-energy iron ions, we used: (1) HRR-deficient rodent cells carrying a deletion in the RAD51D gene and (2) syngeneic human cells impaired for HRR by RAD51D or RAD51 knockdown using RNA interference. We show that in response to iron ions, HRR contributes to cell survival in rodent cells, and that HRR-deficiency abrogates RAD51 foci formation. Complementation of the HRR defect by human RAD51D rescues both enhanced cytotoxicity and RAD51 foci formation. For human cells irradiated with iron ions, cell survival is decreased, and, in p53 mutant cells, the levels of mutagenesis are increased when HRR is impaired. Human cells synchronized in S phase exhibit more pronounced resistance to iron ions as compared with cells in G1 phase, and this increase in radioresistance is diminished by RAD51 knockdown. These results implicate a role for RAD51-mediated DNA repair (i.e. HRR) in removing a fraction of clustered lesions induced by charged particle irradiation. Our results are the first to directly show the requirement for an intact HRR pathway in human cells in ensuring DNA repair and cell survival in response to high-energy high LET radiation.

Study and realisation of an ion source obtained by electronic bombardment - experimentation with phosphorus

International Nuclear Information System (INIS)

Schneider, Philippe

1979-01-01

This research thesis reports the study and development of an ion source by electronic bombardment. In order to solve some practical difficulties (cathode destruction, source instability, and so on), the design of each component has been very careful, notably for the electron gun. The author first briefly discusses the exiting ionisation processes, gives a list of ion which can be produced, with a focus on phosphorus for which the ionisation cross section is defined and assessed. After an assessment of different ionisation processes, and an indication of performance of the best existing sources, the author explains the choice for a totally different process. In the second part, he describes the experimental device, and particularly the electron gun as its design has been an important part of this research work. The source operation is described and its characteristics and performance are studied. Finally, the author outlines that some improvements are still possible to obtain a totally exploitable source [fr

A quadrupole ion trap as low-energy cluster ion beam source

CERN Document Server

Uchida, N; Kanayama, T

2003-01-01

Kinetic energy distribution of ion beams was measured by a retarding field energy analyzer for a mass-selective cluster ion beam deposition system that uses a quadrupole ion trap as a cluster ion beam source. The results indicated that the system delivers a cluster-ion beam with energy distribution of approx 2 eV, which corresponded well to the calculation results of the trapping potentials in the ion trap. Using this deposition system, mass-selected hydrogenated Si cluster ions Si sub n H sub x sup + were actually deposited on Si(111)-(7x7) surfaces at impact kinetic energy E sub d of 3-30 eV. Observation by using a scanning tunneling microscope (STM) demonstrated that Si sub 6 H sub x sup + cluster ions landed on the surface without decomposition at E sub d =3 eV, while the deposition was destructive at E sub d>=18 eV. (author)

Comparison of models of high energy heavy ion collision

International Nuclear Information System (INIS)

Gyulassy, M.

1977-01-01

Some of the main theoretical developments on heavy ion collisions at energies (0.1 to 2.0) GeV/nuc are reviewed. The fireball, firestreak, hydrodynamic (1-fluid, 2-fluids), ''row on row'', hard sphere and intranuclear cascades, and classical equations of motion models are discussed in detail. Results are compared to each other and to measured Ne + U → p + X reactions

Rocking-Chair Ammonium-Ion Battery: A Highly Reversible Aqueous Energy Storage System.

Science.gov (United States)

Wu, Xianyong; Qi, Yitong; Hong, Jessica J; Li, Zhifei; Hernandez, Alexandre S; Ji, Xiulei

2017-10-09

Aqueous rechargeable batteries are promising solutions for large-scale energy storage. Such batteries have the merit of low cost, innate safety, and environmental friendliness. To date, most known aqueous ion batteries employ metal cation charge carriers. Here, we report the first "rocking-chair" NH 4 -ion battery of the full-cell configuration by employing an ammonium Prussian white analogue, (NH 4 ) 1.47 Ni[Fe(CN) 6 ] 0.88 , as the cathode, an organic solid, 3,4,9,10-perylenetetracarboxylic diimide (PTCDI), as the anode, and 1.0 m aqueous (NH 4 ) 2 SO 4 as the electrolyte. This novel aqueous ammonium-ion battery demonstrates encouraging electrochemical performance: an average operation voltage of ca. 1.0 V, an attractive energy density of ca. 43 Wh kg -1 based on both electrodes' active mass, and excellent cycle life over 1000 cycles with 67 % capacity retention. Importantly, the topochemistry results of NH 4 + in these electrodes point to a new paradigm of NH 4 + -based energy storage. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

High energy density in matter produced by heavy ion beams

International Nuclear Information System (INIS)

1986-05-01

In this report the activities of the GSI Darmstadt (FRG) during 1985 concerning inertial confinement fusion by heavy ion beams. Short communications and abstracts are presented concerning a Z-pinch experiment, heavy ion pumped lasers and X-ray spectroscopy, the study of ion-ion collisions, a RFQ development and beam transport studies, accelerator theory, targets for SIS/ESR experiments, the rayleigh-Taylor instability, studies on the equation of state for matter under high pressure, as well as the development of computer codes. (HSI)

High energy density physics studies at the facility for antiprotons and ion research: the HEDgeHOB collaboration

International Nuclear Information System (INIS)

Tahir, N.A.; Stoehlker, T.; Geissel, H.; Shutov, A.; Lomonosov, I.V.; Fortov, V.E.; Piriz, A.R.; Redmer, R.; Deutsch, C.

2011-01-01

The forthcoming Facility for Antiprotons and Ion Research (FAIR) at Darmstadt, is going to be a unique accelerator facility that will deliver high quality, strongly bunched, well focused, intense beams of heavy ions that will lead to unprecedented specific power deposition in solid matter. This will generate macroscopic samples of High Energy Density (HED) matter with fairly uniform physical conditions. These samples can be used to study the thermophysical and transport properties of HED matter. Extensive theoretical work has been carried out over the past decade to design numerous dedicated experiments to study HED physics at the FAIR, which has provided the basis for the HEDgeHOB (High Energy Density Matter Generated by Heavy Ion Beams) scientific proposal. This work is still in progress as the feasibility studies for more experimental schemes are being carried out. Another, very important research area that will benefit tremendously from the FAIR facility, is the production of radioactive beams. A superconducting fragment separator, Super-FRS is being designed for the production and separation of rare radioactive isotopes. Unlike the HED targets, the Super-FRS production target should not be destroyed or damaged by the beam, but should remain intact during the long experimental campaign. However, the high level of specific power deposited in the production target by the high intensity ion beam at FAIR, could cause serious problems to the target survival. These HED issues related to the Super-FRS production target are also discussed in the present paper (copyright 2011 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

Formation of a quasi-hollow beam of high-energy heavy ions using a multicell resonance RF deflector

Science.gov (United States)

Minaev, S. A.; Sitnikov, A. L.; Golubev, A. A.; Kulevoy, T. V.

2012-09-01

The generation of matter in an extreme state with precisely measurable parameters is of great interest for contemporary physics. One way of obtaining such a state is to irradiate the end of a hollow cylindrical shell at the center of which a test material is kept at a temperature of several Kelvin by an annular beam of high-energy heavy ions. Under the action of the beam, the shell starts explosively expanding both outwards and inwards, compressing the material to an extremely high pressure without subjecting it to direct heating. A method of producing a hollow cylindrical beam of high-energy heavy ions using a resonance rf deflector is described. The deflection of the beam in two transverse directions by means of an rf electric field allows it to rotate about the longitudinal axis and irradiate an annular domain on the end face of the target.

Advanced Space Power Systems (ASPS): High Specific Energy Li-ion Battery Cells

Data.gov (United States)

National Aeronautics and Space Administration — The goal of this project element is to increase the specific energy of Li-ion battery cells to 265 Wh/kg and the energy density to 500 Wh/L at 10oC while maintaining...

Analysis of retarding field energy analyzer transmission by simulation of ion trajectories

Science.gov (United States)

van de Ven, T. H. M.; de Meijere, C. A.; van der Horst, R. M.; van Kampen, M.; Banine, V. Y.; Beckers, J.

2018-04-01

Retarding field energy analyzers (RFEAs) are used routinely for the measurement of ion energy distribution functions. By contrast, their ability to measure ion flux densities has been considered unreliable because of lack of knowledge about the effective transmission of the RFEA grids. In this work, we simulate the ion trajectories through a three-gridded RFEA using the simulation software SIMION. Using idealized test cases, it is shown that at high ion energy (i.e., >100 eV) the transmission is equal to the optical transmission rather than the product of the individual grid transparencies. Below 20 eV, ion trajectories are strongly influenced by the electric fields in between the grids. In this region, grid alignment and ion focusing effects contribute to fluctuations in transmission with ion energy. Subsequently the model has been used to simulate the transmission and energy resolution of an experimental RFEA probe. Grid misalignments reduce the transmission fluctuations at low energy. The model predicts the minimum energy resolution, which has been confirmed experimentally by irradiating the probe with a beam of ions with a small energy bandwidth.

High-current heavy-ion accelerator system and its application to material modification

International Nuclear Information System (INIS)

Kishimoto, Naoki; Takeda, Yoshihiko; Lee, C.G.; Umeda, Naoki; Okubo, Nariaki; Iwamoto, Eiji

2001-01-01

A high-current heavy-ion accelerator system has been developed to realize intense particle fluxes for material modification. The facility of a tandem accelerator attained 1 mA-class ion current both for negative low-energy ions and positive high-energy ions. The negative ion source of the key device is of the plasma-sputter type, equipped with mutli-cusp magnets and Cs supply. The intense negative ions are either directly used for material irradiation at 60 keV or further accelerated up to 6 MeV after charge transformation. Application of negative ions, which alleviates surface charging, enables us to conduct low-energy high-current irradiation on insulating substrates. Since positive ions above the MeV range are irrelevant for Coulomb repulsion, the facility as a whole meets the needs of high-current irradiation onto insulators over a wide energy range. Application of high flux ions provides technological merits not only for efficient implantation but also for essentially different material kinetics, which may become an important tool of material modification. Other advantages of the system are co-irradiation by intense laser and in-situ detection of kinetic processes. For examples of material modifications, we present nanoparticle fabrication in insulators, and synergistic phenomena by co-irradiation due to ions and photons. (author)

Collisions of low-energy multicharged ions

International Nuclear Information System (INIS)

Phaneuf, R.A.; Crandall, D.H.

1981-01-01

Experimental measurements of cross sections for collisions of multiply charged ions with atoms at the lowest attainable collision energies are reported. Emphasis is on electron capture from hydrogen atoms by multiply charged ions at energies below 1 keV/amu. The principal effort is the development of a merged-ion-atom-beams apparatus for studies down to 1 eV/amu relative energy

Measurements of low energy auroral ions

International Nuclear Information System (INIS)

Urban, A.

1981-01-01

This paper summarizes ion measurements in the energy range 0.1 to 30 keV observed during the campaigns 'Substorm Phenomena' and 'Porcupine'. For a clear survey of the physical processes during extraordinary events, sometimes ion measurements of higher energies are also taken into account. Generally, the pitch angle distributions were isotropic during all flights except some remarkable events. In general the ion and electron flux intensities correlated, but sometimes revealed a spectral anti-correlation. Acceleration of the ions by an electrostatic field aligned parallel to the magnetic field could be identified accompanied by intense electron precipitation. On the other hand deceleration of the ions was observed in other field-aligned current sheets which are indicated by the electron and magnetic field measurements. Temporal successive monoenergetic ion variations pointed to energy dispersion and to the location of the source region at 9 Rsub(E). Furthermore, ion fluxes higher than those of the electrons were measured at pitch angles parallel to the magnetic field. The integral down-going number and energy flux of the ions contributed to the total particle or energy influx between 65% and less than 7% and did not clearly characterize the geophysical launch conditions or auroral activities. (author)

Ion temperature measurement by neutral energy analyzer in high-field tokamak TRIAM-1

Energy Technology Data Exchange (ETDEWEB)