WorldWideScience

Sample records for helium argon atoms

  1. Attainable superheat of argon-helium, argon-neon solutions.

    Science.gov (United States)

    Baidakov, Vladimir G; Kaverin, Aleksey M; Andbaeva, Valentina N

    2008-10-16

    The method of lifetime measurement has been used to investigate the kinetics of spontaneous boiling-up of superheated argon-helium and argon-neon solutions. Experiments were made at a pressure of p = 1.5 MPa and concentrations up to 0.33 mol% in the range of nucleation rates from 10 (4) to 10 (8) s (-1) m (-3). The homogeneous nucleation regime has been distinguished. With good agreement between experimental data and homogeneous nucleation theory in temperature and concentration dependences of the nucleation rate, a systematic underestimation by 0.25-0.34 K has been revealed in superheat temperatures over the saturated line attained by experiment as compared with theoretical values calculated in a macroscopic approximation. The revealed disagreement between theory and experiment is connected with the dependence of the properties of new-phase nuclei on their size.

  2. Stopping Power of Solid Argon for Helium Ions

    DEFF Research Database (Denmark)

    Besenbacher, F.; Bøttiger, Jørgen; Grauersen, O.

    1981-01-01

    By means of the Rutherford-backscattering method, the stopping cross section of solid argon has been measured for 0.5–3 MeV helium ions to an accuracy of not, vert, similar3%. The results agree within the experimental accuracies with our earlier measurements for gaseous argon over the energy region...

  3. Crossed-beam time-of-flight study of metastable helium in collisions with helium, neon and argon

    Energy Technology Data Exchange (ETDEWEB)

    Fiering, K.B.; Ryan, S.R. (Arizona Univ., Tucson (USA). Dept. of Physics); Wing, W.H. (Arizona Univ., Tucson (USA). Dept. of Physics; Arizona Univ., Tucson (USA). Optical Sciences Center)

    1982-11-14

    Absolute velocity-resolved total integral cross sections have been measured for collisions of helium singlet (2/sup 1/S/sub 0/) and triplet (2/sup 3/S/sub 1/) metastable (He*) atoms with ground-state helium, neon, and argon atoms in the thermal velocity range of 1.0-3.5x10/sup 5/ cms/sup -1/. Additional measurements on the He*-Ne system with a large input aperture at the detector to suppress the sensitivity of the apparatus to elastic scattering failed to show the previously predicted sharply rising velocity structure in the inelastic excitation transfer cross sections.

  4. The Erosion of Frozen Argon by Swift Helium Ions

    DEFF Research Database (Denmark)

    Besenbacher, F.; Bøttiger, Jørgen; Graversen, O.

    1981-01-01

    The temperature, energy, and thickness dependence of the erosion rates of frozen argon films when irradiated with 0.1–3 MeV helium ions have been measured. The erosion yields Y are much too high to be explained by the concentional collisional cascade-sputtering theory and are furthermore unequivo......The temperature, energy, and thickness dependence of the erosion rates of frozen argon films when irradiated with 0.1–3 MeV helium ions have been measured. The erosion yields Y are much too high to be explained by the concentional collisional cascade-sputtering theory and are furthermore...

  5. Trapping fermionic and bosonic helium atoms

    NARCIS (Netherlands)

    Stas, R.J.W.

    2005-01-01

    This thesis presents experimental and theoretical work performed at the Laser Centre of the Vrije Universiteit in Amsterdam to study laser-cooled metastable triplet helium atoms. Samples containing about 3x10^8 helium atoms-either fermionic helium-3 atoms, bosonic helium-4 atoms or mixtures thereof

  6. Trapping fermionic and bosonic helium atoms

    NARCIS (Netherlands)

    Stas, R.J.W.

    2005-01-01

    This thesis presents experimental and theoretical work performed at the Laser Centre of the Vrije Universiteit in Amsterdam to study laser-cooled metastable triplet helium atoms. Samples containing about 3x10^8 helium atoms-either fermionic helium-3 atoms, bosonic helium-4 atoms or mixtures thereof

  7. Trapping fermionic and bosonic helium atoms

    NARCIS (Netherlands)

    Stas, R.J.W.

    2005-01-01

    This thesis presents experimental and theoretical work performed at the Laser Centre of the Vrije Universiteit in Amsterdam to study laser-cooled metastable triplet helium atoms. Samples containing about 3x10^8 helium atoms-either fermionic helium-3 atoms, bosonic helium-4 atoms or mixtures

  8. Trapping cold ground state argon atoms.

    Science.gov (United States)

    Edmunds, P D; Barker, P F

    2014-10-31

    We trap cold, ground state argon atoms in a deep optical dipole trap produced by a buildup cavity. The atoms, which are a general source for the sympathetic cooling of molecules, are loaded in the trap by quenching them from a cloud of laser-cooled metastable argon atoms. Although the ground state atoms cannot be directly probed, we detect them by observing the collisional loss of cotrapped metastable argon atoms and determine an elastic cross section. Using a type of parametric loss spectroscopy we also determine the polarizability of the metastable 4s[3/2](2) state to be (7.3±1.1)×10(-39)  C m(2)/V. Finally, Penning and associative losses of metastable atoms in the absence of light assisted collisions, are determined to be (3.3±0.8)×10(-10)  cm(3) s(-1).

  9. Precision spectroscopy of the helium atom

    Institute of Scientific and Technical Information of China (English)

    Shui-ming HU; Zheng-Tian LU; Zong-Chao YAN

    2009-01-01

    Persistent efforts in both theory and experiment have yielded increasingly precise understanding of the helium atom. Because of its simplicity, the helium atom has long been a testing ground for relativistic and quantum electrodynamic effects in few-body atomic systems theoretically and experimentally.Comparison between theory and experiment of the helium spectroscopy in ls2p3pJ can potentially extract a very precise value of the fine structure constant a. The helium atom can also be used to explore exotic nuclear structures. In this paper, we provide a brief review of the recent advances in precision calculations and measurements of the helium atom.

  10. Helium atom scattering from surfaces

    CERN Document Server

    1992-01-01

    High resolution helium atom scattering can be applied to study a number of interesting properties of solid surfaces with great sensitivity and accuracy. This book treats in detail experimental and theoretical aspects ofthis method as well as all current applications in surface science. The individual chapters - all written by experts in the field - are devoted to the investigation of surface structure, defect shapes and concentrations, the interaction potential, collective and localized surface vibrations at low energies, phase transitions and surface diffusion. Over the past decade helium atom scattering has gained widespread recognitionwithin the surface science community. Points in its favour are comprehensiveunderstanding of the scattering theory and the availability of well-tested approximation to the rigorous theory. This book will be invaluable to surface scientists wishing to make an informed judgement on the actual and potential capabilities of this technique and its results.

  11. Management of Liver Cancer Argon-helium Knife Therapy with Functional Computer Tomography Perfusion Imaging.

    Science.gov (United States)

    Wang, Hongbo; Shu, Shengjie; Li, Jinping; Jiang, Huijie

    2016-02-01

    The objective of this study was to observe the change in blood perfusion of liver cancer following argon-helium knife treatment with functional computer tomography perfusion imaging. Twenty-seven patients with primary liver cancer treated with argon-helium knife and were included in this study. Plain computer tomography (CT) and computer tomography perfusion (CTP) imaging were conducted in all patients before and after treatment. Perfusion parameters including blood flows, blood volume, hepatic artery perfusion fraction, hepatic artery perfusion, and hepatic portal venous perfusion were used for evaluating therapeutic effect. All parameters in liver cancer were significantly decreased after argon-helium knife treatment (p liver tissue, but other parameters kept constant. CT perfusion imaging is able to detect decrease in blood perfusion of liver cancer post-argon-helium knife therapy. Therefore, CTP imaging would play an important role for liver cancer management followed argon-helium knife therapy.

  12. Radioactive ions and atoms in superfluid helium

    NARCIS (Netherlands)

    Dendooven, P.G.; Purushothaman, S.; Gloos, K.; Aysto, J.; Takahashi, N.; Huang, W.; Harissopulos, S; Demetriou, P; Julin, R

    2006-01-01

    We are investigating the use of superfluid helium as a medium to handle and manipulate radioactive ions and atoms. Preliminary results on the extraction of positive ions from superfluid helium at temperatures close to 1 K are described. Increasing the electric field up to 1.2 kV/cm did not improve t

  13. Spectroscopic studies of cryogenic fluids: Benzene in argon and helium

    Science.gov (United States)

    Nowak, R.; Bernstein, E. R.

    1987-09-01

    Energy shifts and bandwidths of the 610 vibronic feature of the 1B2u←1A1g optical absorption spectrum of benzene dissolved in supercritical argon and helium, and in liquid argon are reported as a function of pressure, temperature, and density. Benzene/Ar solutions display red shifts of the 610 transition with increasing density but the dependence is found to be nonlinear at high densities. Benzene/He solutions evidence blue shifts of the 610 transition as a function of increasing density which also becomes nonlinear at high densities. Only small spectral shifts are recorded if the density is kept constant and pressure and temperature are varied simultaneously. In addition, a small density independent temperature effect on the transition energy shift is identified. Experimental results are compared to dielectric (Onsager-Böttcher and Wertheim) and quantum statistical mechanical (Schweizer-Chandler) theories of solvent effects on solute absorption energy. Reasonably good agreement between experiment and theory is found only for the benzene/Ar system at relatively low densities. The theory fails to predict energy shifts for both the benzene/He and high density benzene/Ar systems. This result is different from the findings for the benzene/N2 and benzene/C3H8 solutions and can be interpreted qualitatively in terms of competition between dispersive attractive and repulsive interactions as a function of density. The failure of the theory to describe these transition energy shifts is attributed to the omission of explicit repulsive interactions terms in the theoretical models employed.

  14. Argon Nanoclusters with Fivefold Symmetry in Supersonic Gas Jets and Superfluid Helium

    Science.gov (United States)

    Danylchenko, O. G.; Boltnev, R. E.; Khmelenko, V. V.; Kiryukhin, V.; Konotop, O. P.; Lee, D. M.; Krainyukova, N. V.

    2017-04-01

    In this study argon nanoclusters (800 to ˜ 6500 atoms) formed in supersonic gas jets are compared to the nanoclusters stabilized in superfluid helium. High-energy electron and X-ray diffraction methods are utilized. Both techniques allow investigation of isolated clusters. It is shown that the theoretical prediction of the so-called multiply twinned particles with fivefold symmetry, such as icosahedra (ico) and decahedra (dec) is valid in the investigated cluster size interval. Around the point of the expected ico-to-dec size-dependent transformation at a cluster size of ˜ 2000 atoms, hexagonal ico and the statistical distribution of structures with a tendency for dec to replace ico are observed. Kinetic reasons, as well as temperature-related effects, could be responsible for the latter observations.

  15. First principles study of inert-gas (helium, neon, and argon) interactions with hydrogen in tungsten

    Science.gov (United States)

    Kong, Xiang-Shan; Hou, Jie; Li, Xiang-Yan; Wu, Xuebang; Liu, C. S.; Chen, Jun-Ling; Luo, G.-N.

    2017-04-01

    We have systematically evaluated binding energies of hydrogen with inert-gas (helium, neon, and argon) defects, including interstitial clusters and vacancy-inert-gas complexes, and their stable configurations using first-principles calculations. Our calculations show that these inert-gas defects have large positive binding energies with hydrogen, 0.4-1.1 eV, 0.7-1.0 eV, and 0.6-0.8 eV for helium, neon, and argon, respectively. This indicates that these inert-gas defects can act as traps for hydrogen in tungsten, and impede or interrupt the diffusion of hydrogen in tungsten, which supports the discussion on the influence of inert-gas on hydrogen retention in recent experimental literature. The interaction between these inert-gas defects and hydrogen can be understood by the attractive interaction due to the distortion of the lattice structure induced by inert-gas defects, the intrinsic repulsive interaction between inert-gas atoms and hydrogen, and the hydrogen-hydrogen repelling in tungsten lattice.

  16. Ion velocity distribution functions in argon and helium discharges: detailed comparison of numerical simulation results and experimental data

    Science.gov (United States)

    Wang, Huihui; Sukhomlinov, Vladimir S.; Kaganovich, Igor D.; Mustafaev, Alexander S.

    2017-02-01

    Using the Monte Carlo collision method, we have performed simulations of ion velocity distribution functions (IVDF) taking into account both elastic collisions and charge exchange collisions of ions with atoms in uniform electric fields for argon and helium background gases. The simulation results are verified by comparison with the experiment data of the ion mobilities and the ion transverse diffusion coefficients in argon and helium. The recently published experimental data for the first seven coefficients of the Legendre polynomial expansion of the ion energy and angular distribution functions are used to validate simulation results for IVDF. Good agreement between measured and simulated IVDFs shows that the developed simulation model can be used for accurate calculations of IVDFs.

  17. Photoassociation of cold metastable helium atoms

    NARCIS (Netherlands)

    Woestenenk, G.R.

    2001-01-01

    During the last decades the study of cold atoms has grown in a great measure. Research in this field has been made possible due to the development of laser cooling and trapping techniques. We use laser cooling to cool helium atoms down to a temperature of 1 mK and we are able to tr

  18. Photoassociation of cold metastable helium atoms

    NARCIS (Netherlands)

    Woestenenk, G.R.

    2001-01-01

    During the last decades the study of cold atoms has grown in a great measure. Research in this field has been made possible due to the development of laser cooling and trapping techniques. We use laser cooling to cool helium atoms down to a temperature of 1 mK and we are able to

  19. Photoassociation of cold metastable helium atoms

    NARCIS (Netherlands)

    Woestenenk, G.R.

    2001-01-01

    During the last decades the study of cold atoms has grown in a great measure. Research in this field has been made possible due to the development of laser cooling and trapping techniques. We use laser cooling to cool helium atoms down to a temperature of 1 mK and we are able to tr

  20. What is the shape of the helium trimer? A comparison with the neon and argon trimers.

    Science.gov (United States)

    Bressanini, Dario; Morosi, Gabriele

    2011-10-13

    Despite its apparent simplicity and extensive theoretical investigations, the issue of what is the shape of the helium trimer is still debated in the literature. After reviewing previous conflicting interpretations of computational studies, we introduce the angle-angle distribution function as a tool to discuss in a simple way the shape of any trimer. We compute this function along with many different geometrical distributions using variational and diffusion Monte Carlo methods. We compare them with the corresponding ones for the neon and argon trimers. Our analysis shows that while Ne(3) and Ar(3) fluctuate around an equilibrium structure that is an equilateral triangle, (4)He(3) shows an extremely broad angle-angle distribution function, and all kinds of three-atom configurations must be taken into account in its description. Classifying (4)He(3) as either equilateral or linear or any other particular shape, as was done in the past, is not sensible, because in this case the intuitive notion of equilibrium structure is ill defined. Our results could help the interpretation of future experiments aimed at measuring the geometrical properties of the helium trimer.

  1. Laser Spectroscopy of Antiprotonic Helium Atoms

    CERN Multimedia

    2002-01-01

    %PS205 %title\\\\ \\\\Following the discovery of metastable antiprotonic helium atoms ($\\overline{p}He^{+} $) at KEK in 1991, systematic studies of their properties were made at LEAR from 1991 to 1996. In the first two years the lifetime of $\\overline{p}He^{+}$ in liquid and gaseous helium at various temperatures and pressures was measured and the effect of foreign gases on the lifetime of these atoms was investigated. Effects were also discovered which gave the antiproton a 14\\% longer lifetime in $^4$He than in $^3$He, and resulted in important differences in the shape of the annihilation time spectra in the two isotopes.\\\\ \\\\Since 1993 laser spectroscopy of the metastable $\\overline{p}He^{+}$ atoms became the main focus of PS205. Transitions were stimulated between metastable and non-metastable states of the $\\overline{p}He^{+}$ atom by firing a pulsed dye laser beam into the helium target every time an identified metastable atom was present (Figure 1). If the laser frequency matched the transition energy, the...

  2. Crossed-beam time-of-flight study of metastable helium in collisions with helium, neon, and argon

    Energy Technology Data Exchange (ETDEWEB)

    Fiering, K.B.

    1981-01-01

    Absolute total integral velocity-resolved cross sections have been measured for collisions of helium singlet (2/sup 1/S/sub 0/) and triplet (2/sup 3/S/sub 1/) metastables with ground-state helium, neon, and argon in the thermal velocity range of 1.0 to 3.5 x 10/sup 5/ cm/sec. Additional measurements on the He/sup +/-Ne system with a large input acceptance angle at the detector failed to show previously predicted sharply-rising velocity structure in the inelastic transfer cross sections. The measurements were taken with a crossed-beam time-of-flight apparatus.

  3. a Crossed-Beam Time-Of Study of Metastable Helium in Collisions with Helium, Neon, and Argon.

    Science.gov (United States)

    Fiering, Kenneth Barratt

    Absolute total integral velocity-resolved cross sections have been measured for collisions of helium singlet (2('1)S(,0)) and triplet (2('3)S(,1)) metastables with ground-state helium, neon, and argon in the thermal velocity range of 1.0-3.5 x 10('5) cm/sec. Additional measurements on the He*-Ne system with a large input acceptance angle at the detector failed to show previously predicted sharply -rising velocity structure in the inelastic transfer cross sections. The measurements were taken with a crossed-beam time-of-flight apparatus.

  4. Cryogenic spray vaporization in high-velocity helium, argon and nitrogen gasflows

    Science.gov (United States)

    Ingebo, Robert D.

    1993-01-01

    Effects of gas properties on cryogenic liquid-jet atomization in high-velocity helium, nitrogen, and argon gas flows were investigated. Volume median diameter, D(sub v.5e), data were obtained with a scattered-light scanning instrument. By calculating the change in spray drop size, -Delta D(sub v.5)(exp 2), due to droplet vaporization, it was possible to calculate D(sub v.5C). D(sub v.5C) is the unvaporized characteristic drop size formed at the fuel-nozzle orifice. This drop size was normalized with respect to liquid-jet diameter, D(sub O). It was then correlated with several dimensionless groups to give an expression for the volume median diameter of cryogenic LN2 sprays. This expression correlates drop size D(sub v.5c) with aerodynamic and liquid-surface forces so that it can be readily determined in the design of multiphase-flow propellant injectors for rocket combustors.

  5. Radiative properties of argon-helium-nitrogen-carbon-cobalt-nickel plasmas used in CNT synthesis

    Science.gov (United States)

    Salem, D.; Hannachi, R.; Cressault, Y.; Teulet, Ph; Béji, L.

    2015-02-01

    This work presents the radiative properties of argon-helium-nitrogen-carbon-nickel-cobalt thermal plasmas by the computation of net emission coefficients (NECs) under the assumption of a local thermodynamic equilibrium and at temperature range 1000-20 000 K. These mixtures were often used in the study of carbon nanotubes (CNTs) synthesis with arc plasma which becomes one of the most useful techniques in terms of flexibility of carbon nanostructures produced with fewer defects. The values of NEC allow estimation of total radiation losses in plasmas, by taking into account the emission radiation resulting from the atomic continuum, the molecular continuum, the atomic lines and some molecular bands. Free-free transitions (Bremsstrahlung) and free-bound (electron-ion recombination), have been considered for the calculation of atomic continuum. For bound-bound transitions, natural, resonance, Van der Waals, Stark and Doppler effects have been taken into account in the calculation of the lines broadenings while the self-absorption of the resonance lines has been treated using their escape factors. Molecular continuum has been only considered for N2, C2 and CN molecules whereas we have only taken into account diatomic systems N2, \\text{N}2+ , CN and C2 for the emission of the molecular bands. The results obtained show that even for low concentrations of Ni and Co in the plasma, the NECs are modified and considerably increase only at a low temperature (T < 8000 K) and the major contribution in the total radiation arises from the lines emission. However, the effect of the thickness of the plasma on plasma radiation has been analysed based on the self absorption phenomenon of resonance lines.

  6. Diffusion behaviors of helium atoms at two Pd grain boundaries

    Institute of Scientific and Technical Information of China (English)

    XIA Ji-xing; HU Wang-yu; YANG Jian-yu; AO Bing-yun

    2006-01-01

    The diffusion behaviors of helium atoms at two symmetric grain boundaries (Σ5{210} and Σ3 {112}) of Pd were investigated using molecular dynamics simulations through an analytical embedded-atom method(MAEAM) model. The simulations demonstrate that the interstitial helium atoms are easily trapped at the grain boundaries and precipitated into clusters. Due to the closed-shell electronic configurations of both helium and palladium,Pd grain boundaries yield strong capability of retaining helium atoms. By calculating the mean square displacements(MSD) of an interstitial helium atom at the grain boundaries,the diffusion coefficients were determined,and the linear fits to Arrhenius relation. The diffusion activation energies of interstitial helium atom at these two Pd grain boundaries were also evaluated.

  7. Application of argon-helium cryoablation in resection of intracranial tumors

    Directory of Open Access Journals (Sweden)

    Yu-hao ZHOU

    2017-07-01

    Full Text Available Objective To summarize the curative effect of argon-helium cryoablation in resection of intracranial tumors.  Methods and Results A total of 11 patients with primary intracranial tumors, including 7 cases of glioma and 4 cases of meningioma, were enrolled in this study. The tumor was located in left frontal lobe in 4 cases, left fronto-parietal lobe in 2 cases, left temporal lobe in 2 cases and right temporo-parietal lobe in 3 cases. Argon-helium cryoablation was used to assist intracranial tumor resection. Among 7 cases of glioma, 4 cases were totally removed and 3 cases were partially resected. Four cases of meningioma were totally removed. The average intraoperative blood loss was 80 ml, and average operation time was 80 min. Postoperative clinical symptoms were improved, and head CT or MRI showed no rebleeding. Patients were followed up for an average of 4 years, and none of them suffered from operation-related or postoperative complications such as intracranial infection, or tumor recurrence.  Conclusions Argon - helium cryoablation is suitable for intracranial tumors with different diameters and in different locations. It is safe and effective, with few operation-related or postoperative complications, less rebleeding and low risk of recurrence, which is a highly efficient and relatively low?cost assistant surgical method. DOI: 10.3969/j.issn.1672-6731.2017.06.011

  8. Helium, neon and argon diffraction from Ru(0001).

    Science.gov (United States)

    Minniti, M; Díaz, C; Fernández Cuñado, J L; Politano, A; Maccariello, D; Martín, F; Farías, D; Miranda, R

    2012-09-05

    We present an experimental and theoretical study of He, Ne and Ar diffraction from the Ru(0001) surface. Close-coupling calculations were performed to estimate the corrugation function and the potential well depth in the atom-surface interaction in all three cases. DFT (density functional theory) calculations, including van der Waals dispersion forces, were used to validate the close-coupling results and to further analyze the experimental results. Our DFT calculations indicate that, in the incident energy range 20-150 meV, anticorrugating effects are present in the case of He and Ar diffraction, whereas normal corrugation is observed with Ne beams.

  9. The Zeeman effect for helium atom

    Institute of Scientific and Technical Information of China (English)

    2002-01-01

    The g-factors of the 23P, 21P, and 33P states of the helium atom are calculated by using the vatiational wave functions constructed from the linear combinations of Slater-type basis sets. The relativistic corrections to order α2(a.u.) and the effect of the motion of the center of mass are treated by using first-order perturbation theory. Most of our predicted results are in good agreement with recent results of Yan and Drake, which were obtained by using the wave functions with doubled Hylleraas coordinates. Based on the analysis of the convergence pattern in our calculation, we believe that our predicted value of the δgL-factor for 33P state in 4He, 2.914 15×10-7, ought to be reasonable and accurate, although there are no corresponding experimental data available in the liteature yet to be compared with.

  10. Harmonic oscillator model for the helium atom

    CERN Document Server

    Carlsen, Martin

    2015-01-01

    A harmonic oscillator model in four dimensions is presented for the helium atom to estimate the distance to the inner and outer electron from the nucleus, the angle between electrons and the energy levels. The method is algebraic and is not based on the choice of correct trial wave function. Three harmonic oscillators and thus three quantum numbers are sufficient to describe the two-electron system. We derive a simple formula for the energy in the general case and in the special case of the Wannier Ridge. For a set of quantum numbers the distance to the electrons and the angle between the electrons are uniquely determined as the intersection between three surfaces. We show that the excited states converge either towards ionization thresholds or towards extreme parallel or antiparallel states and provide an estimate of the ground state energy.

  11. A Study of Confined Helium Atom

    Institute of Scientific and Technical Information of China (English)

    2007-01-01

    The helium atom confined by a spherical parabolic potential well is studied employing the adiabatic hyperspherical approach method. Total energies of the ground and three low-excited states are obtained as a function of the confined potential radii. We find that the energies of a spherical parabolic potential well are in good agreement with those of an impenetrable spherical box for the larger confined potential radius. We find also that the confinement may cause accidental degeneracies between levels with different low-excited states and the inversion of the energy values. The results for the three-dimensional spherical potential well and the two-dimensional disc-like potential well are compared with each other. We find that the energy difference between states in a two-dimensional parabolic potential is also obviously larger than the corresponding levels for a spherical parabolic potential.

  12. Adsorption of Helium Atoms on Two-Dimensional Substrates

    Science.gov (United States)

    Burganova, Regina; Lysogorskiy, Yury; Nedopekin, Oleg; Tayurskii, Dmitrii

    2016-01-01

    The study of the adsorption phenomenon of helium began many decades ago with the discovery of graphite as a homogeneous substrate for the investigation of physically adsorbed monolayer films. In particular, helium monoatomic layers on graphite were found to exhibit a very rich phase diagram. In the present work we have investigated the adsorption phenomenon of helium atoms on graphene and silicene substrates by means of density functional theory with Born-Oppenheimer approximation. Helium-substrate and helium-helium interactions were considered from first principles. Vibrational properties of adsorbed monolayers have been used to explore the stability of the system. This approach reproduces results describing the stability of a helium monolayer on graphene calculated by quantum Monte Carlo (QMC) simulations for low and high coverage cases. However, for the moderate coverage value there is a discrepancy with QMC results due to the lack of helium zero point motion.

  13. Adsorption of Helium Atoms on Two-Dimensional Substrates

    Science.gov (United States)

    Burganova, Regina; Lysogorskiy, Yury; Nedopekin, Oleg; Tayurskii, Dmitrii

    2016-12-01

    The study of the adsorption phenomenon of helium began many decades ago with the discovery of graphite as a homogeneous substrate for the investigation of physically adsorbed monolayer films. In particular, helium monoatomic layers on graphite were found to exhibit a very rich phase diagram. In the present work we have investigated the adsorption phenomenon of helium atoms on graphene and silicene substrates by means of density functional theory with Born-Oppenheimer approximation. Helium-substrate and helium-helium interactions were considered from first principles. Vibrational properties of adsorbed monolayers have been used to explore the stability of the system. This approach reproduces results describing the stability of a helium monolayer on graphene calculated by quantum Monte Carlo (QMC) simulations for low and high coverage cases. However, for the moderate coverage value there is a discrepancy with QMC results due to the lack of helium zero point motion.

  14. Classical helium atom with radiation reaction.

    Science.gov (United States)

    Camelio, G; Carati, A; Galgani, L

    2012-06-01

    We study a classical model of helium atom in which, in addition to the Coulomb forces, the radiation reaction forces are taken into account. This modification brings in the model a new qualitative feature of a global character. Indeed, as pointed out by Dirac, in any model of classical electrodynamics of point particles involving radiation reaction one has to eliminate, from the a priori conceivable solutions of the problem, those corresponding to the emission of an infinite amount of energy. We show that the Dirac prescription solves a problem of inconsistency plaguing all available models which neglect radiation reaction, namely, the fact that in all such models, most initial data lead to a spontaneous breakdown of the atom. A further modification is that the system thus acquires a peculiar form of dissipation. In particular, this makes attractive an invariant manifold of special physical interest, the zero-dipole manifold that corresponds to motions in which no energy is radiated away (in the dipole approximation). We finally study numerically the invariant measure naturally induced by the time-evolution on such a manifold, and this corresponds to studying the formation process of the atom. Indications are given that such a measure may be singular with respect to that of Lebesgue.

  15. Method for laser spectroscopy of metastable pionic helium atoms

    Energy Technology Data Exchange (ETDEWEB)

    Hori, M., E-mail: Masaki.Hori@mpq.mpg.de; Sótér, A.; Aghai-Khozani, H. [Max-Planck-Institut für Quantenoptik (Germany); Barna, D. [CERN (Switzerland); Dax, A. [Paul Scherrer Institut (Switzerland); Hayano, R. S.; Murakami, Y.; Yamada, H. [University of Tokyo, Department of Physics (Japan)

    2015-08-15

    The PiHe collaboration is currently attempting to carry out laser spectroscopy of metastable pionic helium atoms using the high-intensity π{sup −} beam of the ring cyclotron facility of the Paul Scherrer Institute. These atoms are heretofore hypothetical three-body Coulomb systems each composed of a helium nucleus, a π{sup −} occupying a Rydberg state, and an electron occupying the 1s ground state. We briefly review the proposed method by which we intend to detect the laser spectroscopic signal. This complements our experiments on metastable antiprotonic helium atoms at CERN.

  16. Effects of metastable species in helium and argon atmospheric pressure plasma jets (APPJs) on inactivation of periodontopathogenic bacteria

    Science.gov (United States)

    Yoon, Sung-Young; Kim, Kyoung-Hwa; Seol, Yang-Jo; Kim, Su-Jeong; Bae, Byeongjun; Huh, Sung-Ryul; Kim, Gon-Ho

    2016-05-01

    The helium and argon have been widely used as discharge gases in atmospheric pressure plasma jets (APPJs) for bacteria inactivation. The APPJs show apparent different in bullet propagation speed and bacteria inactivation rate apparently vary with discharge gas species. This work shows that these two distinctive features of APPJs can be linked through one factor, the metastable energy level. The effects of helium and argon metastable species on APPJ discharge mechanism for reactive oxygen nitrogen species (RONS) generation in APPJs are investigated by experiments and numerical estimation. The discharge mechanism is investigated by using the bullet velocity from the electric field which is obtained with laser induced fluorescence (LIF) measurement. The measured electric field also applied on the estimation of RONS generation, as electron energy source term in numerical particle reaction. The estimated RONS number is verified by comparing NO and OH densities to the inactivation rate of periodontitis bacteria. The characteristic time for bacteria inactivation of the helium-APPJ was found to be 1.63 min., which is significantly less than that of the argon-APPJ, 12.1 min. In argon-APPJ, the argon metastable preserve the energy due to the lack of the Penning ionization. Thus the surface temperature increase is significantly higher than helium-APPJ case. It implies that the metastable energy plays important role in both of APPJ bullet propagation and bacteria inactivation mechanism.

  17. Geochemistry on mantle-derived volatiles in natural gases from eastern China oil/gas provinces (I )——Helium, argon and hydrocarbons in mantle volatiles

    Institute of Scientific and Technical Information of China (English)

    徐永昌; 沈平; 陶明信; 刘文汇

    1997-01-01

    Researches on helium, argon, carbon dioxide and methane are very significant in studies of mantle substance characteristics and mantle evolution. A < -shaped pattern of the isotope composition distribution of helium and argon sourced from the mantle and the crust, abundance distribution, isotopic composition and reservoir formation of carbon dioxide, and mantle-sourced methane are discussed.

  18. Variational calculations of coupling of an incident helium atom to a slab of superfluid helium four

    Energy Technology Data Exchange (ETDEWEB)

    Campbell, C.E.; Halley, J.W.; Hoon, S. [and others

    1995-04-01

    In previous work on the interaction of single helium atoms with a slab of superfluid helium the authors found a large amplitude, dependent on the condensate fraction, for transmission with re-emission of a helium atom at the other side of the slab. Here they report a variational formulation of the problem which permits a time dependent calculation and which does not require any perturbation expansion. The variational principle involves a minimization of the expectation value of the square of the difference H-E. They will present preliminary results of a variational Monte Carlo calculation using a simple variational form for the wave function.

  19. Study of Neutron-Induced Ionization in Helium and Argon Chamber Gases

    CERN Document Server

    Indurthy, D; Harris, D; Kopp, S; Proga, M; Zwaska, R M

    2004-01-01

    Ion chambers used to monitor the secondary hadron and tertiary muon beam in the NuMI neutrino beamline will be exposed to background particles, including low energy neutrons produced in the beam dump. To understand these backgrounds, we have studied Helium- and Argon-filled ionization chambers exposed to intense neutron fluxes from PuBe neutron sources ($E_n=1-10$ MeV). The sources emit about 10$^8$ neutrons per second. The number of ion pairs in the chamber gas volume per incident neutron is derived. While limited in precision because of a large gamma ray background from the PuBe sources, our results are consistent with the expectation that the neutrons interact purely elastically in the chamber gas.

  20. Development of a helium cryostat for laser spectroscopy of atoms with unstable nuclei in superfluid helium

    Energy Technology Data Exchange (ETDEWEB)

    Imamura, Kei, E-mail: kimamura@riken.jp [Department of Physics, Meiji University, 1-1-1 Higashi-Mita, Tama, Kawasaki, Kanagawa 214-8571 (Japan); Furukawa, Takeshi [Department of Physics, Tokyo Metropolitan University, 1-1 Minami-Osawa, Hachioji, Tokyo 192-0397 (Japan); RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Wakui, Takashi [Cyclotron and Radioisotope Center, Tohoku University, 6-3 Aoba, Aramaki, Aoba, Sendai, Miyagi 980-8578 (Japan); Yang, Xiaofei [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); School of Physics, Peking University, Chengfu Road, Haidian District, Beijing 100871 (China); Yamaguchi, Yasuhiro [Department of Physics, Meiji University, 1-1-1 Higashi-Mita, Tama, Kawasaki, Kanagawa 214-8571 (Japan); Tetsuka, Hiroki [Department of Physics, Tokyo Gakugei University, 4-1-1 Nukuikitamachi, Koganei, Tokyo 184-8501 (Japan); Mitsuya, Yosuke [Department of Physics, Meiji University, 1-1-1 Higashi-Mita, Tama, Kawasaki, Kanagawa 214-8571 (Japan); Tsutsui, Yoshiki [Department of Physics, Tokyo Gakugei University, 4-1-1 Nukuikitamachi, Koganei, Tokyo 184-8501 (Japan); Fujita, Tomomi [Department of Physics, Osaka University, 1-1 Machikaneyama, Toyonaka, Osaka 560-0043 (Japan); Ebara, Yuta; Hayasaka, Miki [Department of Physics, Tokyo Gakugei University, 4-1-1 Nukuikitamachi, Koganei, Tokyo 184-8501 (Japan); Arai, Shino; Muramoto, Sosuke [Department of Physics, Meiji University, 1-1-1 Higashi-Mita, Tama, Kawasaki, Kanagawa 214-8571 (Japan); Ichikawa, Yuichi [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Department of Physics, Tokyo Instutute of Technology, 2-12-1 Ookayama, Meguro, Tokyo 152-8551 (Japan); Ishibashi, Yoko [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Department of Physics, University of Tsukuba, 1-1-1 Tennodai, Tsukuba, Ibaraki 305-8577 (Japan); and others

    2013-12-15

    We are developing a new nuclear laser spectroscopic technique for the study of nuclear structure that can be applied to short-lived low-yield atoms with unstable nuclei. The method utilizes superfluid helium (He II) as a trapping medium for high-energy ion beams. A liquid helium cryostat with optical windows is a key apparatus for this type of experiment. We describe the design and the performance of the cryostat which is developed for the present project.

  1. General mechanism for helium blistering involving displaced atom transport

    Energy Technology Data Exchange (ETDEWEB)

    McDonell, W.R.

    1979-01-01

    A mechanism developed to account for formation of vertically elongated blisters in high displacement environments produced by /sup 252/Cf alpha particles and fission fragments has been extended to formation of done-shaped blisters in the low displacement environments produced by simple helium ion beams. In this mechanism, transport of displaced atoms to relieve compressive stresses in the helium-implanted layer allows interconnections of small, subsurface bubbles to form the blister cavity. The same transport may cause thickening of the blister caps at low implantation energies. The transition from dome-shaped to vertically elongated blistering occurs between the 300 and 3000 displacements per helium atom produced by simple helium ions and /sup 252/Cf radiations respectively.

  2. Corrections to the Nonrelativistic Ground Energy of a Helium Atom

    Institute of Scientific and Technical Information of China (English)

    段一士; 刘玉孝; 张丽杰

    2004-01-01

    Considering the nuclear motion, we present the nonrelativistic ground energy of a helium atom by using a simple effective variational wavefunction with a flexible parameter k. Based on the result, the relativistic and radiative corrections to the nonrelativistic Hamiltonian are discussed. The high precision value of the helium ground energy is evaluated to be -2.90338 a.u. With the relative error 0.00034%.

  3. Helium and Argon Isotopes in Spinel Lherzolite from Damaping,Northern Zhangjiakou

    Institute of Scientific and Technical Information of China (English)

    张建珍; 杜建国; 等

    1999-01-01

    Spinel lhezolite found in Damaping,northern Zhangjiakou,Hebei Province occurs as xenoliths in the Hannuoba basalts that consist of alkali basalt and tholeiite.Spinel lherzolites contain50%-70% olivine(Fo:90%),10%-20% clinopyroxene(predominantly Di),10%-30% orthopyroxene(predominantly En),and less than 5%spinl ,3He/4He and 40Ar/38Ar ratios in the olivine are 7.56×10-7and 299.1 respectively,3He/4He and 40Ar/38Ar ratios in the orthopyroxene(enstatite)are 9.1×10-7and 307,respectively,Olivine grains are fractured irregularly,and pyroxene grains characterized by well developed cleavages,which would have resulted from explosion during the rapid eruption of lava from the deep interior to the surface.The lower isotope ratios of helium and argon may indicate that the spinel lherzolite xenoliths were derived from the strongly degassed and depleted upper mantle,and that the mantle is inhomogeneous.3He losses to some extent might affect the helium isotope ratios.

  4. Shift and broadening of resonance lines of antiprotonic helium atoms in solid helium

    CERN Document Server

    Adamczak, Andrzej

    2014-01-01

    We have estimated the shift and broadening of the resonance lines in the spectrum of antiprotonic helium atoms $\\bar{p}\\mathrm{He}^{+}$ implanted in solid helium $^4$He. The application of the response function for crystalline helium has enabled determination of the contributions from the collective degrees of freedom to the shift and broadening. It occurs that the broadening due to the collective motion is negligible compared to the natural line width. The available pair-correlation functions for crystalline $^4$He have been applied for estimating the resonance-line shift due to collisions of $\\bar{p}\\mathrm{He}^{+}$ atom with the surrounding $^4$He atoms. The dependence of the line shift, which has been calculated in the quasistatic limit, on the solid-$^4$He density is nonlinear.

  5. Four-Parameter Scheme for Ground Level of Helium Atom

    Institute of Scientific and Technical Information of China (English)

    HU Xian-Quan; XU Jie; MA Yong; ZHENG Rui-Lun

    2006-01-01

    In this paper, the ground state wave function of four parameters is developed and the expression of the ground state level is derived for the helium atom when the radial Schrodinger equation of the helium atom is solved.The ground energy is respectively computed by the optimized algorithms of Matlab 7.0 and the Monte Carlo methods.Furthermore, the ground state wave function is obtained. Compared with the experiment value and the value with the variation calculus in reference, the results of this paper show that in the four-parameter scheme, not only the calculations become more simplified and precise, but also the radial wave function of the helium atom meets the space symmetry automatically in ground state.

  6. Electronically excited rubidium atom in a helium cluster or film

    Science.gov (United States)

    Leino, Markku; Viel, Alexandra; Zillich, Robert E.

    2008-11-01

    We present theoretical studies of helium droplets and films doped with one electronically excited rubidium atom Rb∗ (P2). Diffusion and path integral Monte Carlo approaches are used to investigate the energetics and the structure of clusters containing up to 14 helium atoms. The surface of large clusters is approximated by a helium film. The nonpair additive potential energy surface is modeled using a diatomic in molecule scheme. Calculations show that the stable structure of Rb∗Hen consists of a seven helium atom ring centered at the rubidium, surrounded by a tirelike second solvation shell. A very different structure is obtained when performing a "vertical Monte Carlo transition." In this approach, a path integral Monte Carlo equilibration starts from the stable configuration of a rubidium atom in the electronic ground state adsorbed to the helium surface after switching to the electronically excited surface. In this case, Rb∗Hen relaxes to a weakly bound metastable state in which Rb∗ sits in a shallow dimple. The interpretation of the results is consistent with the recent experimental observations [G. Auböck et al., Phys. Rev. Lett. 101, 035301 (2008)].

  7. An investigation of high fractions of metastable helium atoms

    Institute of Scientific and Technical Information of China (English)

    X.P.Feng(冯贤平); B.W.James

    2003-01-01

    Penning type discharge was adopted to excite helium atoms. It is suitable for generating high densitymetastables at a range from 0.1 mTorr to 0.5 Tort. The highest metastable density of 3.5 × 1010 cm-3was observed at a static gas pressure of 0.5 Torr. The highest fraction of metastables (N21s/NHe) of 10-3in a low gas pressure was obtained. The variation of the magnetic field strength on the discharge doesnot result in a significant density change of the metastable helium atoms. When no magnetic field wasapplied, no discharge took place.

  8. Using Uncertainty Principle to Find the Ground-State Energy of the Helium and a Helium-like Hookean Atom

    Science.gov (United States)

    Harbola, Varun

    2011-01-01

    In this paper, we accurately estimate the ground-state energy and the atomic radius of the helium atom and a helium-like Hookean atom by employing the uncertainty principle in conjunction with the variational approach. We show that with the use of the uncertainty principle, electrons are found to be spread over a radial region, giving an electron…

  9. Using Uncertainty Principle to Find the Ground-State Energy of the Helium and a Helium-like Hookean Atom

    Science.gov (United States)

    Harbola, Varun

    2011-01-01

    In this paper, we accurately estimate the ground-state energy and the atomic radius of the helium atom and a helium-like Hookean atom by employing the uncertainty principle in conjunction with the variational approach. We show that with the use of the uncertainty principle, electrons are found to be spread over a radial region, giving an electron…

  10. Conversion of an atomic to a molecular argon ion and low pressure argon relaxation

    Science.gov (United States)

    M, N. Stankov; A, P. Jovanović; V, Lj Marković; S, N. Stamenković

    2016-01-01

    The dominant process in relaxation of DC glow discharge between two plane parallel electrodes in argon at pressure 200 Pa is analyzed by measuring the breakdown time delay and by analytical and numerical models. By using the approximate analytical model it is found that the relaxation in a range from 20 to 60 ms in afterglow is dominated by ions, produced by atomic-to-molecular conversion of Ar+ ions in the first several milliseconds after the cessation of the discharge. This conversion is confirmed by the presence of double-Gaussian distribution for the formative time delay, as well as conversion maxima in a set of memory curves measured in different conditions. Finally, the numerical one-dimensional (1D) model for determining the number densities of dominant particles in stationary DC glow discharge and two-dimensional (2D) model for the relaxation are used to confirm the previous assumptions and to determine the corresponding collision and transport coefficients of dominant species and processes. Project supported by the Ministry of Education, Science and Technological Development of the Republic of Serbia (Grant No. ON171025).

  11. The Helium Atom and Isoelectronic Ions in Two Dimensions

    Science.gov (United States)

    Patil, S. H.

    2008-01-01

    The energy levels of the helium atom and isoelectronic ions in two dimensions are considered. The difficulties encountered in the analytical evaluation of the perturbative and variational expressions for the ground state, promote an interesting factorization of the inter-electronic interaction, leading to simple expressions for the energy. This…

  12. Measurement of strong interaction effects in antiprotonic helium atoms

    Energy Technology Data Exchange (ETDEWEB)

    Davies, J.D.; Gorringe, T.P.; Lowe, J.; Nelson, J.M.; Playfer, S.M.; Pyle, G.J.; Squier, G.T.A. (Birmingham Univ. (UK). Dept. of Physics); Baker, C.A.; Batty, C.J.; Clark, S.A.

    1984-09-27

    The strong interaction shift and width for the 2 p level and the width for the 3d level have been measured for antiprotonic helium atoms. The results are compared with optical model calculations. The possible existence of strongly bound antiproton states in nuclei is discussed.

  13. Resonances of the helium atom in a strong magnetic field

    DEFF Research Database (Denmark)

    Lühr, Armin Christian; Al-Hujaj, Omar-Alexander; Schmelcher, Peter

    2007-01-01

    We present an investigation of the resonances of a doubly excited helium atom in a strong magnetic field covering the regime B=0–100  a.u. A full-interaction approach which is based on an anisotropic Gaussian basis set of one-particle functions being nonlinearly optimized for each field strength...

  14. The Helium Atom and Isoelectronic Ions in Two Dimensions

    Science.gov (United States)

    Patil, S. H.

    2008-01-01

    The energy levels of the helium atom and isoelectronic ions in two dimensions are considered. The difficulties encountered in the analytical evaluation of the perturbative and variational expressions for the ground state, promote an interesting factorization of the inter-electronic interaction, leading to simple expressions for the energy. This…

  15. Interactions of satellite-speed helium atoms with satellite-surfaces. 1. Spatial distributions of reflected helium atoms

    Energy Technology Data Exchange (ETDEWEB)

    Liu, S.M.; Rodgers, W.E.; Knuth, E.L.

    1975-06-01

    Interactions of satellite-speed helium atoms with practical satellite surfaces were investigated experimentally, and spatial distributions of satellite-speed helium beams scattered from four different engineering surfaces were measured. The 7000-m/s helium beams were produced using an arc-heated supersonic molecular beam source. The test surfaces included cleaned 6061-T6 aluminum plate, anodized aluminum foil, white paint, and quartz surfaces. Both in-plane (in the plane containing the incident beam and the surface normal) and out-of-plane spatial distributions of reflected helium atoms were measured for six different incidence angles (0, 15, 30, 45, 60, and 75 deg from the surface normal). It was found that a large fraction of the incident helium atoms were scattered back in the vicinity of the incoming beam, particularly in the case of glancing incidence angles. This unexpected scattering feature results perhaps from the gross roughness of these test surfaces. This prominent backscattering could yield drag coefficients which are higher than for surfaces with either forward-lobed or diffusive (cosine) scattering patterns. (auth)

  16. A canine model of osteonecrosis of the femoral head induced by MRI guided argon helium cryotherapy system

    Science.gov (United States)

    Wang, Dong; Sun, Lixin; Zhang, Huawu; Jiang, Honglei; Liu, Ming; Tian, Jing; Hu, Na; Sun, Shui

    2015-01-01

    Objective: This study is to identify the reliability of osteonecrosis of the femoral head (ONFH) modeling established by MRI guided argon helium cryotherapy system in beagles. Methods: A total of 15 beagles were used to establish the ONFH model. The left femoral heads of the beagles received two cycles of argon helium freezing-thawing under MRI guidance and were considered as experimental group while the right femoral heads received only one cycle of argon helium freezing-thawing and were considered as the control group. X-ray, MRI, general shape and histological examinations were performed so as to identify the effect of modeling. Results: At 4 week after modeling, MRI showed obvious bilateral hip joint effusion and marked femoral head bone marrow high signal. At 8 week after surgery, abnormal signal appeared in bilateral femoral heads. T1WI showed irregular patchy low signal, T2WI showed irregular mixed signals and the joint capsule effusion showed long T1 and T2 changes. Twelve weeks after operation, T1WI showed a low signal strip with clear boundary and T2WI showed intermediate signal. The changes of the left femoral heads were significant while compared with those of the right sides. The lacunae rates of femoral heads in the experimental group at 4, 8, and 12 week after surgery (40.75 ± 3.77, 57.46 ± 4.01, 50.27 ± 2.98) were higher than those in control group (30.08 ± 3.61, 49.43 ± 2.82, 40.56 ± 2.73). Conclusion: Canine model of ONFH was successfully established using an argon helium cryotherapy system. PMID:26550205

  17. Atom-atom excitation in shock waves in argon-oxygen mixture

    Energy Technology Data Exchange (ETDEWEB)

    Ezumi, Hiromichi; Kawamura, Masahiko

    1987-05-01

    The slope constants of the excitational cross-section for atom-atom and atom-electron collisions were generally considered and that for the oxygen atom-atom collision S/sub 0-0/ was determined to be 3.14 x 10/sup -19/ cm/sup 2//eV. Using the newly determined value of S/sub 0-0/, the calculation of the ionizing shock structure of argon-oxygen mixture was made at shock Mach number M/sub S/ = 17.1 and the initial pressure P/sub 1/ = 2.85 Torr. From the comparison of the calculated value of relaxation length with the experimental one, it was proved that the experimental result can be explained well by the present determined value of S/sub 0-0/.

  18. Helium and argon isotopic compositions of the Longquanzhan gold deposit in the Yishu fault zone and their geological implications

    Institute of Scientific and Technical Information of China (English)

    2007-01-01

    The Longquanzhan gold deposit hosted in granitic cataclasites with mylontization of the foot wall of the main Yishui-Tangtou fault. 3He/4He ratios in fluid inclusions range from 0.14 to 0.24 R/Ra,close to those of the crust-source helium. 40Ar/36Ar ratios were measured to be 289-1811, slightly higher than those of atmospheric argon. The results of analysis of helium and argon isotopes suggested that ore-forming fluids were derived chiefly from the crust. The δ18O values of fluid inclusions from vein quartz range from -1.78‰ to 4.07‰, and the δD values of the fluid inclusions vary between -74‰ and -77‰. The hydrogen and oxygen isotope data indicated that the ore-forming fluid for the Longquanzhan gold deposit had mixed with meteoric water in the process of mineralization. This is consistent with the conclusion from the helium and argon isotope data.

  19. Inelastic collisions of excited helium atoms with normal rubidium atoms

    Energy Technology Data Exchange (ETDEWEB)

    Blagoev, K.B.; Kasyanenko, S.V.; Krauze, U.; Tolmachev, Y.A.

    1986-05-01

    The afterglow of helium lines in a helium--rubidium mixture excited by a pulsed electron beam has been studied. The effective quenching probabilities at different concentrations of rubidium have been measured, and the rate constants and effective quenching cross sections have been determined. An analysis of possible mechanisms of an inelastic collision is given. A major role of the ionic term in the interaction of the particles during collisions is indicated. The experimental values of the cross sections are compared with the results of a calculation in different approximations.

  20. Field Ionization detection of supersonic helium atom beams

    Science.gov (United States)

    Doak, R. B.

    2003-10-01

    Field ionization detectors (FID) may offer near-unity detection efficiency and nanoscale spatial resolution. To date, FID detection of molecular beams has been limited to effusive beams of broad Maxwellian velocity distributions. We report FID measurements on monoenergetic helium beams, including intensity measurements and time-of-flight measurements. The FID tips were carefully prepared and characterized in a field ionization microscope prior to use. With the supersonic helium beam we find a much smaller effective detection area ( 50 sq. nm) than was reported in the effusive helium beam experiments ( 200,000 sq. nm). This suggests that the FID ionization yield depends strongly on energy loss by the impinging atom during its initial collision with the FID surface: Our thermal energy, monoenergetic helium beam atoms likely lose little or no energy upon scattering from the clean tungsten FID surface, allowing the scattered atoms to escape the FID polarization field and therby reducing the ionization yield. To improve signal levels, inelastic scattering might be enhanced by use of lower beam velocities (present in the tails of a Maxwellian) or by adsorbing an overlayer on the FID tip (present at cryogenic tip temperatures). These factors likely explain the higher detection yields measured in the effusive beam experiments.

  1. On the size and structure of helium snowballs formed around charged atoms and clusters of noble gases.

    Science.gov (United States)

    Bartl, Peter; Leidlmair, Christian; Denifl, Stephan; Scheier, Paul; Echt, Olof

    2014-09-18

    Helium nanodroplets doped with argon, krypton, or xenon are ionized by electrons and analyzed in a mass spectrometer. HenNgx(+) ions containing up to seven noble gas (Ng) atoms and dozens of helium atoms are identified; the high resolution of the mass spectrometer combined with advanced data analysis make it possible to unscramble contributions from isotopologues that have the same nominal mass but different numbers of helium or Ng atoms, such as the magic He20(84)Kr2(+) and the isobaric, nonmagic He41(84)Kr(+). Anomalies in these ion abundances reveal particularly stable ions; several intriguing patterns emerge. Perhaps most astounding are the results for HenAr(+), which show evidence for three distinct, solid-like solvation shells containing 12, 20, and 12 helium atoms. This observation runs counter to the common notion that only the first solvation shell is solid-like but agrees with calculations by Galli et al. for HenNa(+) [J. Phys. Chem. A 2011, 115, 7300] that reveal three shells of icosahedral symmetry. HenArx(+) (2 ≤ x ≤ 7) ions appear to be especially stable if they contain a total of n + x = 19 atoms. A sequence of anomalies in the abundance distribution of HenKrx(+) suggests that rings of six helium atoms are inserted into the solvation shell each time a krypton atom is added to the ionic core, from Kr(+) to Kr3(+). Previously reported strong anomalies at He12Kr2(+) and He12Kr3(+) [Kim , J. H.; et al. J. Chem. Phys. 2006, 124, 214301] are attributed to a contamination. Only minor local anomalies appear in the distributions of HenXex(+) (x ≤ 3). The distributions of HenKr(+) and HenXe(+) show strikingly similar, broad features that are absent from the distribution of HenAr(+); differences are tentatively ascribed to the very different fragmentation dynamics of these ions.

  2. Ultracold metastable helium: Ramsey fringes and atom interferometry

    Science.gov (United States)

    Vassen, W.; Notermans, R. P. M. J. W.; Rengelink, R. J.; van der Beek, R. F. H. J.

    2016-12-01

    We report on interference studies in the internal and external degrees of freedom of metastable triplet helium atoms trapped near quantum degeneracy in a 1.5 μm optical dipole trap. Applying a single π /2 rf pulse we demonstrate that 50% of the atoms initially in the m=+1 state can be transferred to the magnetic field insensitive m=0 state. Two π /2 pulses with varying time delay allow a Ramsey-type measurement of the Zeeman shift for a high precision measurement of the 2 ^3S_1-2 ^1S_0 transition frequency. We show that this method also allows strong suppression of mean-field effects on the measurement of the Zeeman shift, which is necessary to reach the accuracy goal of 0.1 kHz on the absolute transition frequencies. Theoretically the feasibility of using metastable triplet helium atoms in the m=0 state for atom interferometry is studied demonstrating favorable conditions, compared to the alkali atoms that are used traditionally, for a non-QED determination of the fine structure constant.

  3. Imprints from the solar cycle on the helium atom and helium pickup ion distributions

    Directory of Open Access Journals (Sweden)

    D. Rucinski

    Full Text Available Neutral interstellar helium atoms penetrate into the solar system almost unaffected by gas–plasma interactions in the heliospheric interface region, and thus can be considered as carriers of original information on the basic parameters (like density, temperature, bulk velocity of the Very Local Interstellar Medium (VLISM. Such information can nowadays be derived from analysis of data obtained from different experimental methods: in situ measurements of He atoms (Ulysses, observations of the solar backscattered He 584 A radiation (EUVE, in situ measurements of He + pickup ions (AMPTE, Ulysses, Wind, SOHO, ACE. In view of the current coordinated international ISSI campaign devoted to the study of the helium focusing cone structure and its evolution, we analyze expected variations of neutral He density, of He + pickup fluxes and of their phase space distributions at various phases of the solar activity cycle based on a realistic time-dependent modelling of the neutral helium and He + pickup ion distributions, which reflect solar cycle-induced variations of the photoionization rate. We show that the neutral helium density values are generally anticorrelated with the solar activity phase and in extreme cases (near the downwind axis the maximum-to-minimum density ratio may even exceed factors of ~ 3 at 1 AU. We also demonstrate that in the upwind hemisphere (at 1 AU and beyond the He + fluxes are correlated with the solar cycle activity, whereas on the downwind side the maximum of the expected flux up to distances of ~ 3 AU occurs around solar minimum epoch, and only further away does the correlation with solar activity become positive. Finally, we present the response of the phase space distribution spectra of He + pickup ions (in the solar wind frame for different epochs of the solar cycle and heliocentric distances from 1 to 5 AU covering the range of Ulysses, Wind and ACE observations.

    Key words. Solar physics, astrophysics and astronomy

  4. Behavior of Excited Argon Atoms in Inductively Driven Plasmas

    CERN Document Server

    Hebner, G A

    1999-01-01

    Laser induced fluorescence has been used to measure the spatial distribution of the two lowest energy argon excited states, 1s sub 5 and 1s sub 4 , in inductively driven plasmas containing argon, chlorine and boron trichloride. The behavior of the two energy levels with plasma conditions was significantly different, probably because the 1s sub 5 level is metastable and the 1s sub 4 level is radiatively coupled to the ground state but is radiation trapped. The argon data is compared with a global model to identify the relative importance of processes such as electron collisional mixing and radiation trapping. The trends in the data suggest that both processes play a major role in determining the excited state density. At lower rfpower and pressure, excited state spatial distributions in pure argon were peaked in the center of the discharge, with an approximately Gaussian profile. However, for the highest rfpowers and pressures investigated, the spatial distributions tended to flatten in the center of the disch...

  5. A calculation of internal kinetic energy and polarizability of compressed argon from the statistical atom model

    NARCIS (Netherlands)

    Seldam, C.A. ten; Groot, S.R. de

    From Jensen's and Gombás' modification of the statistical Thomas-Fermi atom model, a theory for compressed atoms is developed by changing the boundary conditions. Internal kinetic energy and polarizability of argon are calculated as functions of pressure. At 1000 atm. an internal kinetic energy of

  6. Electronic Relaxation Processes of Transition Metal Atoms in Helium Nanodroplets

    Science.gov (United States)

    Kautsch, Andreas; Lindebner, Friedrich; Koch, Markus; Ernst, Wolfgang E.

    2014-06-01

    Spectroscopy of doped superfluid helium nanodroplets (He_N) gives information about the influence of this cold, chemically inert, and least interacting matrix environment on the excitation and relaxation dynamics of dopant atoms and molecules. We present the results from laser induced fluorescence (LIF), photoionization (PI), and mass spectroscopy of Cr and Cu doped He_N. From these results, we can draw a comprehensive picture of the complex behavior of such transition metal atoms in He_N upon photo-excitation. The strong Cr and Cu ground state transitions show an excitation blueshift and broadening with respect to the bare atom transitions which can be taken as indication for the solvation inside the droplet. From the originally excited states the atoms relax to energetically lower states and are ejected from the He_N. The relaxation processes include bare atom spin-forbidden transitions, which clearly bears the signature of the He_N influence. Two-color resonant two-photon ionization (2CR2PI) also shows the formation of bare atoms and small Cr-He_n and Cu-He_n clusters in their ground and metastable states ^c. Currently, Cr dimer excitation studies are in progress and a brief outlook on the available results will be given. C. Callegari and W. E. Ernst, Helium Droplets as Nanocryostats for Molecular Spectroscopy - from the Vacuum Ultraviolet to the Microwave Regime, in Handbook of High-Resolution Spectroscopy, eds. M. Quack and F. Merkt, John Wiley & Sons, Chichester, 2011. A. Kautsch, M. Koch, and W. E. Ernst, J. Phys. Chem. A, 117 (2013) 9621-9625, DOI: 10.1021/jp312336m F. Lindebner, A. Kautsch, M. Koch, and W. E. Ernst, Int. J. Mass Spectrom. (2014) in press, DOI: 10.1016/j.ijms.2013.12.022 M. Koch, A. Kautsch, F. Lackner, and W. E. Ernst, submitted to J. Phys. Chem. A

  7. Quantum reflection of helium atom beams from a microstructured grating

    OpenAIRE

    Zhao, Bum Suk; Schulz, Stephan A.; Meek, Samuel A.; Meijer, Gerard; Schöllkopf, Wieland

    2008-01-01

    We observe high-resolution diffraction patterns of a thermal-energy helium-atom beam reflected from a microstructured surface grating at grazing incidence. The grating consists of 10-$\\mu$m-wide Cr strips patterned on a quartz substrate and has a periodicity of 20 $\\mu$m. Fully-resolved diffraction peaks up to the $7^{\\rm th}$ order are observed at grazing angles up to 20 mrad. With changes in de Broglie wavelength or grazing angle the relative diffraction intensities show significant variati...

  8. Non-sequential double ionization of helium-like atom

    Institute of Scientific and Technical Information of China (English)

    2001-01-01

    In this paper, author investigated the effect of the Coulomb potential of the core of atomic helium on the rescattering processes. Through the calculation author concluded that the Coulomb potential effect may not play an important role in causing the discrepancy between the experimental data and theoretical results of Kuchievs model, and the NS ionization is dependent on the frequency of the laser field. Furthermore, it is concluded that the strength of the laser field and the charge number of the core affect the frequency regime corresponding to the peak value of the NS ionization rate.

  9. Vacuum polarization in the ground states of bi-muonic helium atoms

    Science.gov (United States)

    Frolov, Alexei M.

    2004-11-01

    The energies and bound-state properties of the bi-muonic helium-3 and helium-4 atoms in their ground 11(S = 0)-states are determined to very high accuracy. It is shown that the lowest order QED (and relativistic) effects play a significantly larger role in the case of bi-muonic 3Heμ2 and 4Heμ2 atoms than in the two-electron He-atoms. In particular, the effect of vacuum polarization and corresponding energy shifts for the ground 11(S = 0)-states in the bi-muonic helium-3 and helium-4 atoms have been evaluated.

  10. Interactions of satellite-speed helium atoms with satellite surfaces. 2: energy distributions of reflected helium atoms. [7000 m/s

    Energy Technology Data Exchange (ETDEWEB)

    Liu, S.M.; Knuth, E.L.

    1976-04-01

    Energy transfer in collisions of satellite-speed (7,000 m/s) helium atoms with a cleaned 6061-T6 satellite-type aluminum surface was investigated by use of the molecular-beam technique. The amount of energy transferred was determined from the measured energy of the molecular-beam and the measured spatial and energy distributions of the reflected atoms. Spatial distributions of helium atoms scattered from a 6061-T6 aluminum surface were measured. The scattering pattern exhibits a prominent backscattering, probably due to the gross surface roughness and/or the relative lattice softness of the aluminum surface. Energy distributions of reflected helium atoms from the same surface were measured for six different incidence angles. For each incidence angle, distributions were measured at approximately sixty scattering positions. At a given scattering position, the energy spectra of the reflected helium atoms and the background gas were obtained by use of the retarding-field energy analyzer. (auth)

  11. Electron localizability indicators ELI and ELIA: the case of highly correlated wavefunctions for the argon atom.

    Science.gov (United States)

    Bezugly, Viktor; Wielgus, Pawel; Wagner, Frank R; Kohout, Miroslav; Grin, Yuri

    2008-06-01

    Electron localizability indicators based on the same-spin electron pair density and the opposite-spin electron pair density are studied for correlated wavefunctions of the argon atom. Different basis sets and reference spaces are used for the multireference configuration interaction method following the complete active space calculations aiming at the understanding of the effect of local electron correlation when approaching the exact wavefunction. The populations of the three atomic shells of Ar atom in real space are calculated for each case.

  12. Modified morphology of graphene sheets by Argon-atom bombardment: molecular dynamics simulations.

    Science.gov (United States)

    Wei, Xiao-Lin; Zhang, Kai-Wang; Wang, Ru-Zhi; Liu, Wen-Liang; Zhong, Jian-Xin

    2011-12-01

    By a molecular dynamics method, we simulated the process of Argon-atom bombardment on a graphene sheet with 2720 carbon atoms. The results show that, the damage of the bombardment on the graphene sheet depends not only on the incident energy but also on the particle flux density of Argon atoms. To compare and analyze the effect of the incident energy and the particle flux density in the Argon-atom bombardment, we defined the impact factor on graphene sheet by calculating the broken-hole area. The results indicate that, there is an exponential accumulated-damage for the impact of both the incident energy and the particle flux density and there is a critical incident energy ranging from 20-30 eV/atom in Argon-atom bombardment. Different configurations, such as sieve-like and circle-like graphene can be formed by controlling of different particle flux density as the incident energy is more than the critical value. Our results supply a feasible method on fabrication of porous graphene-based materials for gas-storages and molecular sieves, and it also helps to understand the damage mechanism of graphene-based electronic devices under high particle radiation.

  13. Quantum reflection of helium atom beams from a microstructured grating

    Science.gov (United States)

    Zhao, Bum Suk; Schulz, Stephan A.; Meek, Samuel A.; Meijer, Gerard; Schöllkopf, Wieland

    2008-07-01

    We observe high-resolution diffraction patterns of a thermal-energy helium atom beam reflected from a microstructured surface grating at grazing incidence. The grating consists of 10-μm -wide Cr strips patterned on a quartz substrate and has a periodicity of 20μm . Fully resolved diffraction peaks up to the seventh order are observed at grazing angles up to 20mrad . With changes in de Broglie wavelength or grazing angle the relative diffraction intensities show significant variations which shed light on the nature of the atom-surface interaction potential. The observations are explained in terms of quantum reflection at the long-range attractive Casimir-van der Waals potential.

  14. Quantum reflection of helium atom beams from a microstructured grating

    CERN Document Server

    Zhao, Bum Suk; Meek, Samuel A; Meijer, Gerard; Schöllkopf, Wieland

    2008-01-01

    We observe high-resolution diffraction patterns of a thermal-energy helium-atom beam reflected from a microstructured surface grating at grazing incidence. The grating consists of 10-$\\mu$m-wide Cr strips patterned on a quartz substrate and has a periodicity of 20 $\\mu$m. Fully-resolved diffraction peaks up to the $7^{\\rm th}$ order are observed at grazing angles up to 20 mrad. With changes in de Broglie wavelength or grazing angle the relative diffraction intensities show significant variations which shed light on the nature of the atom-surface interaction potential. The observations are explained in terms of quantum reflection at the long-range attractive Casimir-van der Waals potential.

  15. Electronic Structure of Helium Atom in a Quantum Dot

    Science.gov (United States)

    Saha, Jayanta K.; Bhattacharyya, S.; Mukherjee, T. K.

    2016-03-01

    Bound and resonance states of helium atom have been investigated inside a quantum dot by using explicitly correlated Hylleraas type basis set within the framework of stabilization method. To be specific, precise energy eigenvalues of bound 1sns (1Se) (n = 1-6) states and the resonance parameters i.e. positions and widths of 1Se states due to 2sns (n = 2-5) and 2pnp (n = 2-5) configurations of confined helium below N = 2 ionization threshold of He+ have been estimated. The two-parameter (Depth and Width) finite oscillator potential is used to represent the confining potential due to the quantum dot. It has been explicitly demonstrated that the electronic structural properties become sensitive functions of the dot size. It is observed from the calculations of ionization potential that the stability of an impurity ion within a quantum dot may be manipulated by varying the confinement parameters. A possibility of controlling the autoionization lifetime of doubly excited states of two-electron ions by tuning the width of the quantum cavity is also discussed here. TKM Gratefully Acknowledges Financial Support under Grant No. 37(3)/14/27/2014-BRNS from the Department of Atomic Energy, BRNS, Government of India. SB Acknowledges Financial Support under Grant No. PSW-160/14-15(ERO) from University Grants Commission, Government of India

  16. Allowed and forbidden transitions in artificial hydrogen and helium atoms.

    Science.gov (United States)

    Fujisawa, Toshimasa; Austing, David Guy; Tokura, Yasuhiro; Hirayama, Yoshiro; Tarucha, Seigo

    2002-09-19

    The strength of radiative transitions in atoms is governed by selection rules that depend on the occupation of atomic orbitals with electrons. Experiments have shown similar electron occupation of the quantized energy levels in semiconductor quantum dots--often described as artificial atoms. But unlike real atoms, the confinement potential of quantum dots is anisotropic, and the electrons can easily couple with phonons of the material. Here we report electrical pump-and-probe experiments that probe the allowed and 'forbidden' transitions between energy levels under phonon emission in quantum dots with one or two electrons (artificial hydrogen and helium atoms). The forbidden transitions are in fact allowed by higher-order processes where electrons flip their spin. We find that the relaxation time is about 200 micro s for forbidden transitions, 4 to 5 orders of magnitude longer than for allowed transitions. This indicates that the spin degree of freedom is well separated from the orbital degree of freedom, and that the total spin in the quantum dots is an excellent quantum number. This is an encouraging result for potential applications of quantum dots as basic entities for spin-based quantum information storage.

  17. Inner-shell Annihilation of Positrons in Argon, Iron and Copper Atoms

    CERN Document Server

    Abdel-Raouf, M A; El-Bakry, S Y

    2007-01-01

    The annihilation parameters of positrons with electrons in different shells of Argon, Iron and Copper atoms are calculated below the positronium (Ps) formation thresholds. Quite accurate ab initio calculations of the bound state wavefunctions of Argon, Iron and Copper orbitals are obtained from Cowan computer code. A least-squares variational method (LSVM) is used for determining the wavefunction of the positrons. The program is employed for calculating the s-wave partial cross sections of positrons scattered by Iron and Copper atoms. Our results of the effective charge are compared with available experimental and theoretical ones. --

  18. Photoionization Spectroscopy of Isolated cr Atoms in Ultracold Helium Nanodroplets

    Science.gov (United States)

    Kautsch, Andreas; Hasewend, Matthias; Ratschek, Martin; Koch, Markus; Ernst, Wolfgang E.

    2012-06-01

    Recently we succeeded in doping Cr atoms to He nanodroplets (HeN) at 0.4 Kand carried out resonance ionization mass spectroscopy (RIMS). Here we present resonant two-photon ionization (R2PI) measurements in the wavelength range from 350 to 361 nm (27700 - 28600 cm-1, 3.43 - 3.54 eV). As one of several possible ionization pathways we allocate a first excitation step to the y7Po ← a7S3 transition, happening inside the HeN. Due to the interaction with the surrounding He this excitation appears broadened in the spectra and gives the possibility to obtain detailed information about the perturbation upon electronic excitation of the Cr atom in HeN. Subsequently, the dopant atom leaves the HeN and is ionized in the gas phase where discrete free atom autoionization levels are populated leading to additional sharp spectral features. Future investigations with two photon two color ionization and selective electron energy ionization as well as quantum chemistry calculations will be discussed. M. Ratschek, M. Koch, and W. E. Ernst, J. Chem. Phys., in press (2012) C. Callegari and W. E. Ernst, Helium Droplets as Nanocryostats for Molecular Spectroscopy - from the Vacuum Ultraviolet to the Microwave Regime, in Handbook of High-Resolution Spectroscopy, eds. M. Quack and F. Merkt, John Wiley & Sons, Chichester, 2011.

  19. A novel animal model of osteonecrosis of the femoral head induced using a magnetic resonance imaging-guided argon-helium cryotherapy system

    Science.gov (United States)

    WANG, DONG; WANG, GUOWEI; LIU, MING; SUN, LIXIN; ZONG, WEI; JIANG, HONGLEI; ZHANG, HUAWU; LI, HUIBO; GONG, JIANBAO; SUN, SHUI

    2014-01-01

    The aim of the present study was to establish a novel animal model of osteonecrosis of the femoral head (ONFH) using a magnetic resonance imaging (MRI)-guided argon-helium cryotherapy system. A total of 48 rabbits were used to generate the ONFH models. In group I, the left femoral head of the rabbits received two cycles of argon-helium freezing-thawing under MRI guidance, while in group II, the right femoral head of each rabbit received only one cycle of argon-helium freezing-thawing. X-ray and histological examinations were performed. The percentages of lacunae in the femoral heads of group I at weeks 4, 8 and 12 following surgery (49.75±3.17, 62.06±4.12 and 48.25±2.76%, respectively) were higher than those in group II (39.13±4.48, 50.69±3.84 and 37.50±3.86%, respectively). In addition, the percentage of empty lacunae in group I was 62.06% at week 8 following surgery. Therefore, an animal model of ONFH was successfully established using an argon-helium cryotherapy system. The percentage of empty lacunae in group I was higher than that in group II at weeks 4, 8 and 12 after surgery. PMID:24926337

  20. Helium atom scattering investigation of the Sb(111) surface.

    Science.gov (United States)

    Mayrhofer-Reinhartshuber, M; Tamtögl, A; Kraus, P; Ernst, W E

    2013-10-02

    The Sb(111) surface was studied with helium atom scattering (HAS). Elastic HAS at different energies of the incident helium beam (15.3, 21.9, 28.4 meV) was applied for structural investigations. The lattice constants derived from the positions of the observed diffraction peaks up to third order were found to be in perfect agreement with previous structure determinations of Sb(111). The observed diffraction patterns with clear peaks up to second order were used to model the electronic surface corrugation with the GR method. As an estimation for the attractive part of the interaction potential a well depth of (4.0 ± 0.5) meV was found. Best fit results were obtained with a corrugation height of 12-13% of the lattice constant, which is rather large compared to other surfaces with metallic character. Intensity measurements of the specular peak as a function of incident energy were analysed to determine the distribution of terraces on the surface. The results show a quite flat Sb(111) surface and a step height of 3.81 Å of the remaining terraces.

  1. Electronic structure of helium atom in a quantum dot

    CERN Document Server

    Saha, Jayanta K; Mukherjee, T K

    2015-01-01

    Bound and resonance states of helium atom have been investigated inside a quantum dot by using explicitly correlated Hylleraas type basis set within the framework of stabilization method. To be specific, precise energy eigenvalues of bound 1sns (1Se) [n = 1-6] states and the resonance parameters i.e. positions and widths of 1Se states due to 2sns [n = 2-5] and 2pnp [n = 2-5] configuration of confined helium below N = 2 ionization threshold of He+ have been estimated. The two-parameter (Depth and Width) finite oscillator potential is used to represent the confining potential representing the quantum dot. It has been explicitly demonstrated that electronic structure properties become a sensitive function of the dot size. It is observed from the calculations of ionization potential that the stability of an impurity ion within quantum dot may be manipulated by varying the confinement parameters. A possibility of controlling the autoionization lifetime of doubly excited states of two-electron ions by tuning the wi...

  2. A study of argon, neon and helium based gas mixtures for improving the spatial resolution in time projection chambers

    Energy Technology Data Exchange (ETDEWEB)

    Alber, T. (Max-Planck-Institut fuer Physik, D-80805, Muenchen (Germany)); Eckardt, V. (Max-Planck-Institut fuer Physik, D-80805, Muenchen (Germany)); Fessler, H. (Max-Planck-Institut fuer Physik, D-80805, Muenchen (Germany)); Schoenfelder, S. (Max-Planck-Institut fuer Physik, D-80805, Muenchen (Germany)); Seyboth, P. (Max-Planck-Institut fuer Physik, D-80805, Muenchen (Germany))

    1994-09-15

    For large TPCs in future experiments at the Large Hadron Collider (LHC, CERN) and at the Relativistic Heavy Ion Collider (RHIC, Brookhaven) it is of great interest to optimize the gas characteristics and the readout geometry for the planned application. For this a large number of argon, neon and helium based gases with CH[sub 4], C[sub 2]H[sub 6] and CO[sub 2] admixtures as quenchers were studied. The drift velocity and the transverse and longitudinal electron diffusion were measured for drift field strengths between 70 and 200 V/cm. Improvements of the readout chambers were tested. Effects on the spatial and the two-track resolution are discussed. ((orig.))

  3. CT assessment of liver hemodynamics in patients with hepatocellular carcinoma after argon-helium cryoablation

    Institute of Scientific and Technical Information of China (English)

    Xue-Jia Hao; Jin-Ping Li; Hui-Jie Jiang; Da-Qing Li; Zai-Sheng Ling

    2013-01-01

    BACKGROUND: Assessment  of  tumor  response  after  argon-helium  cryoablation  is  critical  in  guiding  future  therapy  for unresectable  hepatocellular  carcinoma.  This  study  aimed  to evaluate  liver  hemodynamics  in  hepatocellular  carcinoma after  argon-helium  cryoablation  with  computed  tomography perfusion. METHODS: The  control  group  comprised  40  volunteers without liver disease.  The  experimental  group  was  composed of  15  patients  with  hepatocellular  carcinoma  treated  with argon-helium  cryoablation.  Computed  tomography  perfusion parameters were measured: hepatic blood flow, hepatic blood volume,  mean  transit  time,  permeability  of  capillary  vessel surface, hepatic arterial fraction, hepatic arterial perfusion, and hepatic portal perfusion. RESULTS: After  treatment,  in  the  tumor  foci,  permeability of  capillary  vessel  surface  was  higher,  and  hepatic  blood flow,  hepatic  blood  volume,  hepatic  arterial  fraction,  and hepatic  arterial  perfusion  values  were  lower  (P0.05). CONCLUSION: Computed tomography perfusion can evaluate tumor response after argon-helium cryoablation.

  4. A Helium Atom Confined by a Spherical Gaussian Potential Well

    Institute of Scientific and Technical Information of China (English)

    QIU Liang; XIE Wen-Fang; WANG An-Min

    2008-01-01

    The helium atom confined by a non-impenetrable spherical box, i.e., a spherical Gaussian potential well which possesses finite height and range, is studied employing the exact diagonalization method. Total energies of the ground and three low-excited states are obtained as a function of the confined potential radii. We find that the confinement may cause accidental degeneracies between levels with different low-excited states and the inversion of the energy values. The results for the three-dimensional spherical potential well and the two-dimensional disc-like potential well are compared with each other: in general, the energies of the states decrease and the energy intervals between states increase with the reduction of the space dimensions.

  5. Relativistic Corrections to the Zeeman Effect of Helium Atom

    Institute of Scientific and Technical Information of China (English)

    关晓旭; 李白文; 王治文

    2002-01-01

    The high-order relativistic corrections to the Zeeman g-factors of the helium atom are calculated. AII the relativistic correction terms and the term describing the motion of the mass centre are treated as perturbations. Most of our results are in good agreement with those of Yah and Drake [Phys. Rev. A 50 (1994)R1980/, who used the wavefunctions constructed by Hylleraas coordinates. For the correction δg of the g-factor of the 3 3P state in 4He, our result, 2.91415 × 10-7 a.u., should be more reasonable and accurate, although there are no experimental data available in the literature to compare.

  6. Reactions of pulsed laser produced boron and nitrogen atoms in a condensing argon stream

    Science.gov (United States)

    Andrews, Lester; Hassanzadeh, Parviz; Burkholder, Thomas R.; Martin, J. M. L.

    1993-01-01

    Reactions of pulsed laser produced B and N atoms at high dilution in argon favored diboron species. At low laser power with minimum radiation, the dominant reaction with N2 gave BBNN (3Π). At higher laser power, reactions of N atoms contributed the B2N (2B2), BNB (2Σu+), NNBN (1Σ+), and BNBN (3Π) species. These new transient molecules were identified from mixed isotopic patterns, isotopic shifts, and ab initio calculations of isotopic spectra.

  7. Semiclassical calculation of ionisation rate for Rydberg helium atoms in an electric field

    Institute of Scientific and Technical Information of China (English)

    Wang De-Hua

    2011-01-01

    The ionisation of Rydberg helium atoms in an electric field above the classical ionisation threshold has been examined using the semiclassical method, with particular emphasis on discussing the influence of the core scattering on the escape dynamics of electrons. The results show that the Rydberg helium atoms ionise by emitting a train of electron pulses. Unlike the case of the ionisation of Rydberg hydrogen atom in parallel electric and magnetic fields,where the pulses of the electron are caused by the external magnetic field, the pulse trains for Rydberg helium atoms are created through core scattering. Each peak in the ionisation rate corresponds to the contribution of one core-scattered combination trajectory. This fact further illustrates that the ionic core scattering leads to the chaotic property of the Rydberg helium atom in external fields. Our studies provide a simple explanation for the escape dynamics in the ionisation of nonhydrogenic atoms in external fields.

  8. Bubble growth from clustered hydrogen and helium atoms in tungsten under a fusion environment

    Science.gov (United States)

    You, Yu-Wei; Kong, Xiang-Shan; Wu, Xuebang; Liu, C. S.; Chen, J. L.; Luo, G.-N.

    2017-01-01

    Bubbles seriously degrade the mechanical properties of tungsten and thus threaten the safety of nuclear fusion devices, however, the underlying atomic mechanism of bubble growth from clustered hydrogen and helium atoms is still mysterious. In this work, first-principles calculations are therefore carried out to assess the stability of tungsten atoms around both hydrogen and helium clusters. We find that the closest vacancy-formation energies of interstitial hydrogen and helium clusters are substantially decreased. The first-nearest and second-nearest vacancy-formation energies close to vacancy-hydrogen clusters decrease in a step-like way to  ˜0, while those close to vacancy-helium clusters are reduced almost linearly to  ˜-5.46 eV when atom number reaches 10. The vacancy-formation energies closest to helium clusters are more significantly reduced than those nearest to hydrogen clusters, whatever the clusters are embedded at interstitial sites or vacancies. The reduction of vacancy-formation energies results in instability and thus emission of tungsten atoms close to interstitial helium and vacancy-helium clusters, which illustrates the experimental results, that the tungsten atoms can be emitted from the vicinity of vacancy-helium clusters. In addition, the emission of unstable tungsten atoms close to hydrogen clusters may become possible once they are disturbed by the environment. The emission of tungsten atoms facilitates the growth and evolution of hydrogen and helium clusters and ultimately the bubble formation. The results also explain the bubble formation even if no displacement damage is produced in tungsten exposed to low-energy hydrogen and helium plasma.

  9. X-ray observation of a helium atom and placing a nitrogen atom inside He@C60 and He@C70.

    Science.gov (United States)

    Morinaka, Yuta; Sato, Satoru; Wakamiya, Atsushi; Nikawa, Hidefumi; Mizorogi, Naomi; Tanabe, Fumiyuki; Murata, Michihisa; Komatsu, Koichi; Furukawa, Ko; Kato, Tatsuhisa; Nagase, Shigeru; Akasaka, Takeshi; Murata, Yasujiro

    2013-01-01

    Single crystal X-ray analysis has been used as a powerful method to determine the structure of molecules. However, crystallographic data containing helium has not been reported, owing to the difficulty in embedding helium into crystalline materials. Here we report the X-ray diffraction study of He@C60 and the clear observation of a single helium atom inside C60. In addition, the close packing of a helium atom and a nitrogen atom inside fullerenes is realized using two stepwise insertion techniques, that is, molecular surgery to synthesize the fullerenes encapsulating a helium atom, followed by nitrogen radio-frequency plasma methods to generate the fullerenes encapsulating both helium and nitrogen atoms. Electron spin resonance analysis reveals that the encapsulated helium atom has a small but detectable influence on the electronic properties of the highly reactive nitrogen atom coexisting inside the fullerene, suggesting the potential usage of helium for controlling electronic properties of reactive species.

  10. Effect of carbon and alloying solute atoms on helium behaviors in α-Fe

    Science.gov (United States)

    Zhang, Yange; You, Yu-Wei; Xu, Yichun; Liu, C. S.; Chen, J. L.; Luo, G.-N.

    2017-02-01

    Helium bubbles could strongly degrade the mechanical properties of ferritic steels in fission and fusion systems. The formation of helium bubble is directly affected by the interactions between helium and the compositions in steels, such as solute atoms, carbon and irradiation defects. We thereby performed systematical first-principles calculations to investigate the interactions of solute-helium and carbon-solute-helium. It is found that substitutional helium is more attractive than interstitial helium to all the considered 3p, 4p, 5p and 6p solutes. The attraction between carbon and substitutional helium suggests the carbon-solute-helium complex can be formed stably. By examining the charge density difference and thermal stability, it is found that the ternary complex shows stronger attraction with He than that of solute-helium pair for some solutes (S, Se, In, Te, Pb and Bi) and the complex could existed in iron stably at 700 K. The present theoretical results may be helpful for exploring alloy additions to mitigate the formation of large helium bubbles.

  11. On the origins of trapped helium, neon and argon isotopic variations in meteorites. I - Gas-rich meteorites, lunar soil and breccia. II - Carbonaceous meteorites.

    Science.gov (United States)

    Black, D. C.

    1972-01-01

    Data are presented from stepwise heating experiments and total extractions on five meteorites: Kapoeta, Fayetteville, Holman Island, Cee Vee, and Pultusk. These data reveal the presence of four isotopically distinct trapped neon components. A comparison of trapped neon with trapped helium and argon in bulk analyses indicates the existence of correlated helium, neon and argon isotopic structures. Component B is attributed primarily to direct implantation of rare gas ions by the present day solar wind. Component C is identified with directly implanted low energy (1-10 Mev/n) solar flare rare gases. Component D is associated with rare gas ions implanted in meteoritic material by the primitive, pre-main sequence, solar wind. A fourth component, observed only in Kapoeta and the lunar fines and breccia, is tentatively attributed to parent body 'atmospheric' ions implanted in surface material by a solar wind induced electric field.

  12. Vacuum polarization in the ground states of bi-muonic helium atoms

    Energy Technology Data Exchange (ETDEWEB)

    Frolov, Alexei M [Department of Chemistry, Queen' s University, Kingston, ON K7L 3N6 (Canada)

    2004-11-28

    The energies and bound-state properties of the bi-muonic helium-3 and helium-4 atoms in their ground 1{sup 1}(S = 0)-states are determined to very high accuracy. It is shown that the lowest order QED (and relativistic) effects play a significantly larger role in the case of bi-muonic {sup 3}He{mu}{sub 2} and {sup 4}He{mu}{sub 2} atoms than in the two-electron He-atoms. In particular, the effect of vacuum polarization and corresponding energy shifts for the ground 1{sup 1}(S 0)-states in the bi-muonic helium-3 and helium-4 atoms have been evaluated.

  13. Clinical Observation on the Combined Treatment of 57 Cases of Non-small Cell Lung Cancer Using Argon-Helium Cryosurgery and Chinese Herbal Medicine

    Institute of Scientific and Technical Information of China (English)

    2007-01-01

    Objective: To observe the clinical effect of the combined therapy using argon-helium cryosurgery (Ar-He knife) and Chinese herbal medicine in treating non-small cell lung cancer (NSCLC).Methods: Fifty-seven patients of NSCLC were treated with the combined therapy and observed. Results:The treatment was successfully completed in all patients with mild adverse reactions. The effective rate was 83.8% 3 months after the operation, 79.6% 6 months after the operation, and 77.3% 12 months after the operation, with median survival of 9 months. The survival rate after 12 months was 46.67%(21/45), 34.62% (9/26) after 18 months, and 36.36% (4/11) after 24 months. Conclusion: Argon-helium cryosurgery therapy is superior in its assured orientation, quick tumor load deprivation and less postoperational reaction. Combined with Chinese herbal medication, Argon-helium cryosurgery therapy can prolong survival time, relieve clinical symptoms, and elevate the quality of life in NSCLC patients, and is thus worthy of promotion.

  14. Unraveling the absorption spectra of alkali metal atoms attached to helium nanodroplets.

    Science.gov (United States)

    Bünermann, Oliver; Droppelmann, Georg; Hernando, Alberto; Mayol, Ricardo; Stienkemeier, Frank

    2007-12-13

    The absorption spectra of the first electronic exited state of alkali metal atoms on helium nanodroplets formed of both 4He and 3He isotopes were studied experimentally as well as theoretically. In the experimental part new data on the 2palkali metal atoms with helium nanodroplets, a model calculation was performed. New helium density profiles as well as a refined model allowed us to achieve good agreement with the experimental findings. For the first time the red-shifted intensities in the lithium and sodium spectra are explained in terms of enhanced binding configurations in the excited state displaced spatially from the ground state configurations.

  15. Helium and argon isotope trace in ore-forming fluid of Sawuer gold belt in Xinjiang, China

    Institute of Scientific and Technical Information of China (English)

    SHEN Ping; SHEN Yuanchao; ZENG Qingdong; LIU Tiebing; LI Guangming

    2004-01-01

    The helium and argon isotope compositions of fluid inclusions hosted in pyrite have been measured from Kuoerzhenkuola and Buerkesidai gold deposits in Sawuer gold belt, northern Xinjiang. The results show that fluidinclusion 3He/4He ratios are 0.64 Ra-4.25 Ra and 1.16 Ra 9.48 Ra, 40Ar/36Ar ratios are 282-359 and 312-525 for Kuoerzhenkuola and Buerkesidai gold deposits respectively.The ore-forming fluids of two deposits possessed the same source and derived mainly from mantle beneath the island arc (including oceanic crust and oceanic sediments by subduction of oceanic plate). They were diluted by incorporating meteoric water to form a mixture of mantle- and partial meteoric water-derived fluid. The ore-forming fluids of two deposits are of the same evolutionary histories. From the early to the late mineralization stages, the ratios of meteoric water/mantle- derived fluid in ore-forming fluid increased gradually. Based on these results and detailed geological and geochemical studies on the two deposits, it is proposed that the geneses of the two gold deposits are the same, being volcanogenic late-stage hydrothermal gold deposits occurring in the same volcanic apparatus.

  16. Effects of discharge current and voltage on the high density of metastable helium atoms

    Institute of Scientific and Technical Information of China (English)

    FengXian-Ping; DAndruczyk; BWJames; KTakiyama; SNamba; TOda

    2003-01-01

    Both hollow-cathode and Penning-type discharges were adopted toexcite helium atoms to a metastable state. Experimental data indicate that Penning discharge is more suitable for generating high fractions of metastables in a low-density helium hean for laser-induced fluorescence technique in measuring electric fields at the edge of a plasma. The metastable density increases with increasing helium gas pressure in the range of 1.33×10-2-66.7Pa. The highest metastable density of 3.8×1016m-3 is observed at a static gas pressure of 66.7Pa. An approximately linear relationship between the density of metastable helium atoms and the plasma discharge current is observed. Magnetic field plays a very important role in producing a high density of metastable atoms in Penning discharge.

  17. Effects of discharge current and voltage on the high density of metastable helium atoms

    Institute of Scientific and Technical Information of China (English)

    Feng Xian-Ping(冯贤平); D Andruczyk; B W James; K Takiyama; S Namba; T Oda

    2003-01-01

    Both hollow-cathode and Penning-type discharges were adopted to excite helium atoms to a metastable state.Experimental data indicate that Penning discharge is more suitable for generating high fractions of metastables in a low-density helium beam for laser-induced fluorescence technique in measuring electric fields at the edge of a plasma.The metastable density increases with increasing helium gas pressure in the range of 1.33× 10-2-66.7Pa. The highest metastable density of 3.8 × 1016m-3 is observed at a static gas pressure of 66.7Pa. An approximately linear relationship between the density of metastable helium atoms and the plasma discharge current is observed. Magnetic field plays a very important role in producing a high density of metastable atoms in Penning discharge.

  18. X-ray fluorescence/Auger-electron coincidence spectroscopy of vacancy cascades in atomic argon

    Energy Technology Data Exchange (ETDEWEB)

    Arp, U. [National Inst. of Standards and Technology, Gaithersburg, MD (United States). Electron and Optical Physics Div.; LeBrun, T.; Southworth, S.H.; Jung, M. [Argonne National Lab., IL (United States). Physics Div.; MacDonald, M.A. [E.P.S.R.C. Daresbury Lab., Warrington (United Kingdom)

    1996-12-01

    Argon L{sub 2.3}-M{sub 2.3}M{sub 2.3} Auger-electron spectra were measured in coincidence with K{alpha} fluorescent x-rays in studies of Ar K-shell vacancy decays at several photon energies above the K-threshold and on the 1s-4p resonance in atomic argon. The complex spectra recorded by conventional electron spectroscopy are greatly simplified when recorded in coincidence with fluorescent x-rays, allowing a more detailed analysis of the vacancy cascade process. The resulting coincidence spectra are compared with Hartree-Fock calculations which include shake-up transitions in the resonant case. Small energy shifts of the coincidence electron spectra are attributed to post-collision interaction with 1s photoelectrons.

  19. Atomically resolved phase transition of fullerene cations solvated in helium droplets

    Science.gov (United States)

    Kuhn, M.; Renzler, M.; Postler, J.; Ralser, S.; Spieler, S.; Simpson, M.; Linnartz, H.; Tielens, A. G. G. M.; Cami, J.; Mauracher, A.; Wang, Y.; Alcamí, M.; Martín, F.; Beyer, M. K.; Wester, R.; Lindinger, A.; Scheier, P.

    2016-11-01

    Helium has a unique phase diagram and below 25 bar it does not form a solid even at the lowest temperatures. Electrostriction leads to the formation of a solid layer of helium around charged impurities at much lower pressures in liquid and superfluid helium. These so-called `Atkins snowballs' have been investigated for several simple ions. Here we form HenC60+ complexes with n exceeding 100 via electron ionization of helium nanodroplets doped with C60. Photofragmentation of these complexes is measured by merging a tunable narrow-bandwidth laser beam with the ions. A switch from red- to blueshift of the absorption frequency of HenC60+ on addition of He atoms at n=32 is associated with a phase transition in the attached helium layer from solid to partly liquid (melting of the Atkins snowball). Elaborate molecular dynamics simulations using a realistic force field and including quantum effects support this interpretation.

  20. Atomic scattering from an adsorbed monolayer solid with a helium beam that penetrates to the substrate

    DEFF Research Database (Denmark)

    Hansen, Flemming Yssing; Bruch, L.W.; Dammann, Bernd

    2013-01-01

    Diffraction and one-phonon inelastic scattering of a thermal energy helium atomic beam are evaluated in the situation that the target monolayer lattice is so dilated that the atomic beam penetrates to the interlayer region between the monolayer and the substrate. The scattering is simulated...

  1. Introduction to Density Functional Theory: Calculations by Hand on the Helium Atom

    Science.gov (United States)

    Baseden, Kyle A.; Tye, Jesse W.

    2014-01-01

    Density functional theory (DFT) is a type of electronic structure calculation that has rapidly gained popularity. In this article, we provide a step-by-step demonstration of a DFT calculation by hand on the helium atom using Slater's X-Alpha exchange functional on a single Gaussian-type orbital to represent the atomic wave function. This DFT…

  2. Introduction to Density Functional Theory: Calculations by Hand on the Helium Atom

    Science.gov (United States)

    Baseden, Kyle A.; Tye, Jesse W.

    2014-01-01

    Density functional theory (DFT) is a type of electronic structure calculation that has rapidly gained popularity. In this article, we provide a step-by-step demonstration of a DFT calculation by hand on the helium atom using Slater's X-Alpha exchange functional on a single Gaussian-type orbital to represent the atomic wave function. This DFT…

  3. Variability of helium, neon, and argon in the lunar exosphere as observed by the LADEE NMS instrument

    Science.gov (United States)

    Benna, M.; Mahaffy, P. R.; Halekas, J. S.; Elphic, R. C.; Delory, G. T.

    2015-05-01

    The Neutral Mass Spectrometer (NMS) onboard the Lunar Atmosphere and Dust Environment Explorer (LADEE) provided the first global characterization of He and Ar along with the discovery of Ne in the lunar exosphere. The mapping of the equatorial distribution of these noble gases revealed new selenographic and temporal variations. Helium was found to be controlled by the supply of solar wind alpha particles and by the presence of an endogenous source that supplies the exosphere at a rate of 1.9 × 1023 atoms s-1. Neon was detected over the nightside at levels comparable to He and was found to exhibit the spatial distribution of a surface accommodated noncondensable gas. The global measurements of NMS revealed the presence of a localized Ar enhancement that has never been identified before at the western maria. The variability resulting from this local enhancement is coupled to a more global but transient source.

  4. Atomic and ionic spectrum lines below 2000A: hydrogen through argon

    Energy Technology Data Exchange (ETDEWEB)

    Kelly, R.L.

    1982-10-01

    A critical tabulation of observed spectral lines below 2000 angstroms has been prepared from the published literature up to July 1978. It is intended principally as an aid to those physicists and astronomers who deal with the spectra of highly stripped atoms. This report includes the first 18 elements, from hydrogen (including deuterium) through argon. The tabulation is divided into two main sections: the spectrum lines by spectrum, and a finding list. The entries for each element give the ionization species, ground state term, and ionization potential, as well as the best values of vacuum wavelength, intensity, and classification. A list of the pertinent references is appended at the end.

  5. Argon 4s and 4p Excited States Atomic Data Applied in ARC-JET Modeling

    Directory of Open Access Journals (Sweden)

    K. Katsonis

    2011-01-01

    Full Text Available Evaluated atomic data concerning the 4s and 4p configurations of Ar I are averaged in order to simplify their use in various cases of Ar plasma modeling and diagnostics. These data are used here to model a low-power arcjet, running with Argon at low pressure. In so doing, they are explicitly introduced in the chemical processes included in a fluid Navier-Stokes type code, allowing for evaluation of the spectroscopically measurable level populations and of the electronic temperatures. The characteristics of the model are described and the main processes are discussed in view of the results of the calculations.

  6. Slurry micro-sampling technique for use in argon-helium microwave induced plasma optical emission spectrometry.

    Science.gov (United States)

    Ślachciński, Mariusz

    2016-12-01

    The Flow Focusing Pneumatic Nebulizer (FFPN) working at low liquid flow rates was evaluated for the elemental analysis in slurried samples by argon-helium microwave induced plasma optical emission spectrometry (MIP-OES). The obtained results achieved were compared with commercially available V-groove Babington type nebulizer (VBPN). A univariate approach and the simplex optimization procedure were used to achieve optimized conditions and derive analytical figures of merit. Analytical performance of the micro nebulization system was characterized by a determination of the limits of detection (LODs), the precision (RSDs) and the wash-out times for Ba, Ca, Cd, Cu, Fe, Mg, Mn, Pb and Sr. The experimental concentration detection limits for simultaneous determination, calculated as the concentration giving a signal equal to three times of the standard deviation of the blank (LOD, 3σblank criterion, peak height) were 0.9, 0.2, 0.3, 0.2, 0.3, 0.1, 0.2, 0.4, 0.4 and 0.3ngmL(-1) for Ba, Ca, Cd, Cu, Fe, Mg, Mn, Pb and Sr, respectively. The method offers relatively good precision (RSD ranged from 5% to 8%) for micro-slurry sampling analysis. Analyses of the certified reference materials (NRCC DOLT-2, GBW 07302 and SRM 2710) were performed in order to determine the accuracy available with the presented nebulization systems. The measured contents of elements in the reference materials were in satisfactory agreement with the certified values. In addition, these elements were determined in two real samples. Slurry concentration up to 3% m/v (particles technique. An ultrasonic probe was used to homogenize the slurry in the polypropylene bottle just before its introduction into the nebulizer. The nebulizers exhibited no clogging problems. Copyright © 2016 Elsevier B.V. All rights reserved.

  7. Helium and argon isotopes of the Tertiary basic igneous rocks from Shandong Peninsula and implications for the magma origin

    Institute of Scientific and Technical Information of China (English)

    2007-01-01

    Helium (He) and Argon (Ar) isotopic compositions of the Tertiary basic igneous rocks were determined by the high temperature melting extraction method. The selected samples for the studies included al-kaline basalts and diabases from the Jiyang basin,and the surrounding Shanwang and Qixia outcrops in the Shandong Peninsula,eastern China. The results show that the Paleogene basalts and diabases from the Jiyang basin yielded a wide range of P4 PHe abundance of (73.70-804.16)×10 P-8 Pcm P3 P STP·g P-1 P,with P3 PHe/ P4 PHe ratios of 0.374-2.959 Ra,which was lower than the MORB but evidently higher than the con-tinental crust value. The Neogene alkaline basalts from the Jiyang basin,Shanwang and Qixia outcrops have variable P4 PHe abundances ((42.34-286.72)×10-8 Pcm P3 P STP·g-1 P),and "continental crust-like" P3 PHe/ P4 PHe ratios (0.013-0.074 Ra). All of them contain atmospheric-like P40 PAr/ P36 PAr ratio (395.4-1312.7),reflecting the mantle sources with air components. Their low P3 PHe/ P4 PHe ratios are interpreted as the enrichment of the radiogenic P4 PHe mainly inherited from the mantle. He and Ar systematics show the mixing of MORB-type,air and a P4 PHe enriched member in the mantle source,suggesting that these igneous rocks originated from the depleted asthenospheric mantle mixed with an EMI component. Therefore,the present He and Ar isotopes do not support the viewpoints that the Cenozoic igneous rocks of Eastern North China were the products of mantle plume(s) activities.

  8. Helium and argon isotopes of the Tertiary basic igneous rocks from Shandong Peninsula and implications for the magma origin

    Institute of Scientific and Technical Information of China (English)

    TANG HuaYun; ZHENG JianPing; CHEN HongHan; YE XianRen

    2007-01-01

    Helium (He) and Argon (Ar) isotopic compositions of the Tertiary basic igneous rocks were determined by the high temperature melting extraction method. The selected samples for the studies included alkaline basalts and diabases from the Jiyang basin, and the surrounding Shanwang and Qixia outcrops in the Shandong Peninsula, eastern China. The results show that the Paleogene basalts and diabases from the Jiyang basin yielded a wide range of 4 He abundance of (73.70-804.16)×10-8 cm3 STP·Gp-1, with 3He/4He ratios of 0.374-2.959 Ra, which was lower than the MORB but evidently higher than the continental crust value. The Neogene alkaline basalts from the Jiyang basin, Shanwang and Qixia outcrops have variable 4He abundances ((42.34-286.72)×10-8 cm3 STP·g-1), and "continental crust-like" 3He/4He ratios (0.013-0.074 Ra). All of them contain atmospheric-like 40Ar/36Ar ratio (395.4-1312.7), reflecting the mantle sources with air components. Their low 3He/4He ratios are interpreted as the enrichment of the radiogenic 4He mainly inherited from the mantle. He and Ar systematics show the mixing of MORB-type, air and a 4He enriched member in the mantle source, suggesting that these igneous rocks originated from the depleted asthenospheric mantle mixed with an EMI component. Therefore, the present He and Ar isotopes do not support the viewpoints that the Cenozoic igneous rocks of Eastern North China were the products of mantle plume(s) activities.

  9. The role of correlation in the ground state energy of confined helium atom

    Energy Technology Data Exchange (ETDEWEB)

    Aquino, N. [Departamento de Física, Universidad Autónoma Metropolitana-Iztapalapa, Apartado Postal 55-534, 09340 México Distrito Federal (Mexico)

    2014-01-14

    We analyze the ground state energy of helium atom confined by spherical impenetrable walls, and the role of the correlation energy in the total energy. The confinement of an atom in a cavity is one way in which we can model the effect of the external pressure on an atom. The calculations of energy of the system are carried out by the variational method. We find that the correlation energy remains almost constant for a range values of size of the boxes analyzed.

  10. Field ionization of free helium atoms: Correlation between the kinetic energy of ionized atoms and probability of their field ionization

    Energy Technology Data Exchange (ETDEWEB)

    Piskur, J.; Borg, L. [Institute of Experimental Physics, Graz University of Technology, Petersgasse 16, 8010 Graz (Austria); Stupnik, A.; Leisch, M. [Institute of Solid State Physics, Graz University of Technology, Petersgasse 16, 8010 Graz (Austria); Ernst, W.E. [Institute of Experimental Physics, Graz University of Technology, Petersgasse 16, 8010 Graz (Austria); Holst, B. [Institute of Experimental Physics, Graz University of Technology, Petersgasse 16, 8010 Graz (Austria)], E-mail: bodil@cantab.net

    2008-05-15

    In this paper the correlation between the kinetic energy of helium atoms and the probability of field ionization is investigated by exploiting the narrow velocity distribution of supersonic molecular beams. Field ionization measurements were carried out on supersonic helium beams at 298 K and 95 K corresponding to energies of about 65 meV and 20 meV, respectively, for the individual atoms. The field ionization was performed with a tungsten tip, radius of curvature 12 nm, kept at room temperature. The ionization probability was found to increase by about a factor 10 when the beam was cooled from 298 K to 95 K. The results presented in this paper are of importance for improving the understanding of field ionization and for the development of a new detector for helium and other molecular beams.

  11. Field ionization of free helium atoms: Correlation between the kinetic energy of ionized atoms and probability of their field ionization

    Science.gov (United States)

    Piskur, J.; Borg, L.; Stupnik, A.; Leisch, M.; Ernst, W. E.; Holst, B.

    2008-05-01

    In this paper the correlation between the kinetic energy of helium atoms and the probability of field ionization is investigated by exploiting the narrow velocity distribution of supersonic molecular beams. Field ionization measurements were carried out on supersonic helium beams at 298 K and 95 K corresponding to energies of about 65 meV and 20 meV, respectively, for the individual atoms. The field ionization was performed with a tungsten tip, radius of curvature 12 nm, kept at room temperature. The ionization probability was found to increase by about a factor 10 when the beam was cooled from 298 K to 95 K. The results presented in this paper are of importance for improving the understanding of field ionization and for the development of a new detector for helium and other molecular beams.

  12. Excitation of hydrogen atoms in collisions with helium atoms: the role of electron–electron interaction

    Science.gov (United States)

    Frémont, F.; Belyaev, A. K.

    2017-02-01

    Cross sections for producing H(nl) excited state atoms in H(1s) + He(1s2) collisions are calculated using the CTMC method, at impact energies ranging from 20 eV to 100 keV. The role of the electron correlation is studied. In the first step, the interactions between each pair of the three electrons are neglected. This leads to disagreement of the calculated total cross section for producing H(2l) atoms with previous experimental and theoretical results. In a second step, the electron–electron interaction is taken into account in a rigorous way, that is, in the form of the pure Coulomb potential. To make sure that the He target is stable before the collision, phenomenological potentials for the electron–helium-nucleus interactions that simulate the Heisenberg principle are included in addition to the Coulomb potential. The excitation cross section calculated in the frame of this model is in remarkable agreement with previous data in the range between 200 eV and 5 keV. At other energies, discrepancies are revealed, but only by a factor of less than 2 at high energies. The present results show the decisive role of the electron–electron interaction during collisions. In addition, they demonstrate the ability of classical mechanics to take into account the effects of the electron correlation.

  13. Absolute number densities of helium metastable atoms determined by atomic absorption spectroscopy in helium plasma-based discharges used as ambient desorption/ionization sources for mass spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    Reininger, Charlotte; Woodfield, Kellie [Brigham Young University, Department of Chemistry and Biochemistry, Provo, UT 84602 (United States); Keelor, Joel D.; Kaylor, Adam; Fernández, Facundo M. [Georgia Institute of Technology, School of Chemistry and Biochemistry, Atlanta, GA 30332 (United States); Farnsworth, Paul B., E-mail: paul_farnsworth@byu.edu [Brigham Young University, Department of Chemistry and Biochemistry, Provo, UT 84602 (United States)

    2014-10-01

    The absolute number densities of helium atoms in the 2s {sup 3}S{sub 1} metastable state were determined in four plasma-based ambient desorption/ionization sources by atomic absorption spectroscopy. The plasmas included a high-frequency dielectric barrier discharge (HF-DBD), a low temperature plasma (LTP), and two atmospheric-pressure glow discharges, one with AC excitation and the other with DC excitation. Peak densities in the luminous plumes downstream from the discharge capillaries of the HF-DBD and the LTP were 1.39 × 10{sup 12} cm{sup −3} and 0.011 × 10{sup 12} cm{sup −3}, respectively. Neither glow discharge produced a visible afterglow, and no metastable atoms were detected downstream from the capillary exits. However, densities of 0.58 × 10{sup 12} cm{sup −3} and 0.97 × 10{sup 12} cm{sup −3} were measured in the interelectrode regions of the AC and DC glow discharges, respectively. Time-resolved measurements of metastable atom densities revealed significant random variations in the timing of pulsed absorption signals with respect to the voltage waveforms applied to the discharges. - Highlights: • We determine He metastable number densities for four plasma types • The highest number densities were observed in a dielectric barrier discharge • No helium metastable atoms were observed downstream from the exits of glow discharges.

  14. Spectroscopy of antiprotonic helium atoms and its contribution to the fundamental physical constants

    CERN Document Server

    Hayano, R S

    2010-01-01

    Proceedings of the Japan Academy, Series B Vol. 86 (2010) No. 1 P 1-10 Language: Next Article http://dx.doi.org/10.2183/pjab.86.1 JST.JSTAGE/pjab/86.1 Reviews Spectroscopy of antiprotonic helium atoms and its contribution to the fundamental physical constants Ryugo S. HAYANO1) 1) Department of Physics, The University of Tokyo Released 2010/01/14 Keywords: antiproton, CERN, fundamental physical constants, laser spectroscopy Full Text PDF [1604K] Abstracts References(25) Antiprotonic helium atom, a metastable neutral system consisting of an antiproton, an electron and a helium nucleus, was serendipitously discovered, and has been studied at CERN’s antiproton decelerator facility. Its transition frequencies have recently been measured to nine digits of precision by laser spectroscopy. By comparing these experimental results with three-body QED calculations, the antiproton-to-electron massratio was determined as 1836.152674(5). This result contributed to the CODATA recommended val...

  15. Resonant two-photon ionization spectroscopy of Al atoms and dimers solvated in helium nanodroplets

    Energy Technology Data Exchange (ETDEWEB)

    Krasnokutski, Serge A.; Huisken, Friedrich [Laboratory Astrophysics Group of the Max Planck Institute for Astronomy at the Friedrich Schiller University Jena, Institute of Solid State Physics, Helmholtzweg 3, D-07743 Jena (Germany)

    2015-02-28

    Resonant two-photon ionization (R2PI) spectroscopy has been applied to investigate the solvation of Al atoms in helium droplets. The R2PI spectra reveal vibrational progressions that can be attributed to Al–He{sub n} vibrations. It is found that small helium droplets have very little chance to pick up an aluminum atom after collision. However, the pick-up probability increases with the size of the helium droplets. The absorption band that is measured by monitoring the ions on the mass of the Al dimer is found to be very little shifted with respect to the Al monomer band (∼400 cm{sup −1}). However, using the same laser wavelength, we were unable to detect any Al{sub n} photoion with n larger than two.

  16. Resonant two-photon ionization spectroscopy of Al atoms and dimers solvated in helium nanodroplets.

    Science.gov (United States)

    Krasnokutski, Serge A; Huisken, Friedrich

    2015-02-28

    Resonant two-photon ionization (R2PI) spectroscopy has been applied to investigate the solvation of Al atoms in helium droplets. The R2PI spectra reveal vibrational progressions that can be attributed to Al-He(n) vibrations. It is found that small helium droplets have very little chance to pick up an aluminum atom after collision. However, the pick-up probability increases with the size of the helium droplets. The absorption band that is measured by monitoring the ions on the mass of the Al dimer is found to be very little shifted with respect to the Al monomer band (∼400 cm(-1)). However, using the same laser wavelength, we were unable to detect any Al(n) photoion with n larger than two.

  17. A Hartree–Fock study of the confined helium atom: Local and global basis set approaches

    Energy Technology Data Exchange (ETDEWEB)

    Young, Toby D., E-mail: tyoung@ippt.pan.pl [Zakład Metod Komputerowych, Instytut Podstawowych Prolemów Techniki Polskiej Akademia Nauk, ul. Pawińskiego 5b, 02-106 Warszawa (Poland); Vargas, Rubicelia [Universidad Autónoma Metropolitana Iztapalapa, División de Ciencias Básicas e Ingenierías, Departamento de Química, San Rafael Atlixco 186, Col. Vicentina, Iztapalapa, D.F. C.P. 09340, México (Mexico); Garza, Jorge, E-mail: jgo@xanum.uam.mx [Universidad Autónoma Metropolitana Iztapalapa, División de Ciencias Básicas e Ingenierías, Departamento de Química, San Rafael Atlixco 186, Col. Vicentina, Iztapalapa, D.F. C.P. 09340, México (Mexico)

    2016-02-15

    Two different basis set methods are used to calculate atomic energy within Hartree–Fock theory. The first is a local basis set approach using high-order real-space finite elements and the second is a global basis set approach using modified Slater-type orbitals. These two approaches are applied to the confined helium atom and are compared by calculating one- and two-electron contributions to the total energy. As a measure of the quality of the electron density, the cusp condition is analyzed. - Highlights: • Two different basis set methods for atomic Hartree–Fock theory. • Galerkin finite element method and modified Slater-type orbitals. • Confined atom model (helium) under small-to-extreme confinement radii. • Detailed analysis of the electron wave-function and the cusp condition.

  18. Laser spectroscopy of the antiprotonic helium atom – its energy levels and state lifetimes

    CERN Document Server

    Hidetoshi, Yamaguchi

    2003-01-01

    The antiprotonic atom is a three-body exotic system consisting of an antiproton, an electron and a helium nucleus. Its surprising longevity was found and has been studied for more than 10 years. In this work, transition energies and lifetimes of this exotic atom were systematically studied by using the antiproton beam of AD(Antiproton Decelerator) facility at CERN, with an RFQ antiproton decelerator, a narrow-bandwidth laser, Cerenkov counters with fast-response photomultiplier tubes, and cryogenic helium target systems. Thirteen transition energies were determined with precisions of better than 200 ppb by a laser spectroscopy method, together with the elimination of the shift effect caused by collisions with surrounding atoms. Fifteen lifetimes (decay rates) of short-lived states were determined from the time distributions of the antiproton-annihilation signals and the resonance widths of the atomic spectral lines. The relation between the magnitude of the decay rates and the transition multipolarity was inv...

  19. Helium,neon and argon isotope compositions of fluid inclu-sions in massive sulfides from the Jade hydrothermal field,the Okinawa Trough

    Institute of Scientific and Technical Information of China (English)

    ZENG Zhigang; QIN Yunshan; ZHAI Shikui

    2004-01-01

    Helium, neon and argon isotope compositions of fluid inclusions have been measured in massive sulfide samples from the Jade hydrothermal field in the central Okinawa Trough. Huid-inclusion 3He/4He ratios are between 6.2 and 10.1 times the air value (Ra), and with a mean of 7.8Ra, which are consistent with the mid-ocean ridge basalt values [3He/4He≈(6Ra~11Ra)]. Values for 20Ne/22Ne are from 10.7 to 11.3, which are significantly higher than the atmospheric ratio (9.8).And the fluid-inclusion 40Ar/36Ar ratios range from 287 to 334, which are close to the atmosperic values (295.5). These results indicate that the noble gases of trapped hydrothermal fluids in massive sulfides are a mixture of mantle- and seawater-derived components, and the helium of fluid inclusions is mainly from mantle, the nelium and argon isotope compositions are mainly from seawater.

  20. Effect of high power CO2 and Yb:YAG laser radiation on the characteristics of TIG arc in atmospherical pressure argon and helium

    Science.gov (United States)

    Wu, Shikai; Xiao, Rongshi

    2015-04-01

    The effects of laser radiation on the characteristics of the DC tungsten inert gas (TIG) arc were investigated by applying a high power slab CO2 laser and a Yb:YAG disc laser. Experiment results reveal that the arc voltage-current curve shifts downwards, the arc column expands, and the arc temperature rises while the high power CO2 laser beam vertically interacts with the TIG arc in argon. With the increase of the laser power, the voltage-current curve of the arc shifts downwards more significantly, and the closer the laser beam impingement on the arc to the cathode, the more the decrease in arc voltage. Moreover, the arc column expansion and the arc temperature rise occur mainly in the region between the laser beam incident position and the anode. However, the arc characteristics hardly change in the cases of the CO2 laser-helium arc and YAG laser-arc interactions. The reason is that the inverse Bremsstrahlung absorption coefficients are greatly different due to the different electron densities of the argon and helium arcs and the different wave lengths of CO2 and YAG lasers.

  1. ELASTIC AND INELASTIC HELIUM ATOM SCATTERING AT A CLEAVED MICA SHEET

    NARCIS (Netherlands)

    BRUSDEYLINS, G; SCHMICKER, D

    1995-01-01

    A mica sheet has been cleaved in situ in a UHV beam scattering apparatus. The diffraction of the helium atoms shows sharp Bragg peaks. In the [110] and [110] directions of the hexagonal surface the intensities of the Bragg peaks are analysed in terms of a sinusoidal corrugation. With hard wall scatt

  2. Excitation of the shear horizontal mode in a monolayer by inelastic helium atom scattering

    DEFF Research Database (Denmark)

    Bruch, L. W.; Hansen, Flemming Yssing

    2005-01-01

    Inelastic scattering of a low-energy atomic helium beam (HAS) by a physisorbed monolayer is treated in the one-phonon approximation using a time-dependent wave,packet formulation. The calculations show that modes with shear horizontal polarization can be excited near high symmetry azimuths...

  3. Variation in the terrestrial isotopic composition and atomic weight of argon

    Science.gov (United States)

    Böhlke, John Karl

    2014-01-01

    The isotopic composition and atomic weight of argon (Ar) are variable in terrestrial materials. Those variations are a source of uncertainty in the assignment of standard properties for Ar, but they provide useful information in many areas of science. Variations in the stable isotopic composition and atomic weight of Ar are caused by several different processes, including (1) isotope production from other elements by radioactive decay (radiogenic isotopes) or other nuclear transformations (e.g., nucleogenic isotopes), and (2) isotopic fractionation by physical-chemical processes such as diffusion or phase equilibria. Physical-chemical processes cause correlated mass-dependent variations in the Ar isotope-amount ratios (40Ar/36Ar, 38Ar/36Ar), whereas nuclear transformation processes cause non-mass-dependent variations. While atmospheric Ar can serve as an abundant and homogeneous isotopic reference, deviations from the atmospheric isotopic ratios in other Ar occurrences limit the precision with which a standard atomic weight can be given for Ar. Published data indicate variation of Ar atomic weights in normal terrestrial materials between about 39.7931 and 39.9624. The upper bound of this interval is given by the atomic mass of 40Ar, as some samples contain almost pure radiogenic 40Ar. The lower bound is derived from analyses of pitchblende (uranium mineral) containing large amounts of nucleogenic 36Ar and 38Ar. Within this interval, measurements of different isotope ratios (40Ar/36Ar or 38Ar/36Ar) at various levels of precision are widely used for studies in geochronology, water–rock interaction, atmospheric evolution, and other fields.

  4. Spectral Analysis and Metastable Absorption Measurements of High Pressure Capacitively and Inductively Coupled Radio-Frequency Argon-Helium Discharges

    Science.gov (United States)

    2013-06-01

    states. The non -statistical nature implies either the equilibrium kinetics of the argon and electrons in the discharge are non - Maxwellian , the pop...and is shown in Figure 16. The clearly non - Maxwellian nature of the population distribution and the exclusion of the higher lying states are the...approaches the non - Maxwellian production and destruction rates of of the argon states in the discharge and is forcing them into a Boltzmann

  5. Higher-order recoil corrections for triplet states of the helium atom

    CERN Document Server

    Patkos, V; Pachucki, K

    2016-01-01

    Nuclear recoil corrections of order $\\alpha^6\\,m^2/M$ are calculated for the lowest-lying triplet states of the helium atom. It improves the theoretical prediction for the isotope shift of the $2^3S-2^3P$ transition energy and influences the determination of the ${}^3\\textrm{He}-{}^4\\textrm{He}$ nuclear charge radii difference. This calculation is a step forward on the way towards the direct determination of the charge radius of the helium nucleus from spectroscopic measurements.

  6. Spectral line shifts of alkali atoms in liquid helium: a relativistic density functional approach

    Energy Technology Data Exchange (ETDEWEB)

    Anton, J [Universitaet Kassel, Institut fuer Physik, 34109 Kassel (Germany); Mukherjee, P K [Indian Association for the Cultivation of Science, Jadavpur, Kolkata-700 032 (India); Fricke, B [Universitaet Kassel, Institut fuer Physik, 34109 Kassel (Germany); Fritzsche, S [Universitaet Kassel, Institut fuer Physik, 34109 Kassel (Germany)

    2007-06-28

    Excitation line shifts of the principal resonance transitions in alkali atoms sodium and cesium embedded inside the liquid helium environment have been calculated using four-component relativistic density functional theory. The effect of the liquid helium environment is assumed to be represented by a cluster of 14 atoms surrounding the central alkali atom. The estimated blue shift of the principal resonance line {sup 2}S {yields}{sup 2}P is 22.8 nm for Na and 16.7 nm for Cs. The result for Cs is in good agreement with the experimental shift of 18.2 nm. In the absence of the experimental data for Na, our result is compared with those of other theoretical estimates.

  7. Theoretical and experimental study of the Stark effect in the ground state of alkali atoms in helium crystals

    OpenAIRE

    2007-01-01

    This thesis work describes a detailed study of the Stark interaction in the ground state of cesium atoms trapped in a solid helium matrix. The motivation for the investigation of electric field effects on alkali species implanted in solid helium is related to the original main goal of our experimental activities, i.e., the measurement of a permanent atomic electric dipole moment (EDM). The existence of an atomic EDM simultaneously violates the discrete symmetries of time reversal (T) and pari...

  8. Effect of 800 keV argon ions pre-damage on the helium blister formation of tungsten exposed to 60 keV helium ions

    Energy Technology Data Exchange (ETDEWEB)

    Chen, Zhe; Han, Wenjia; Yu, Jiangang; Zhu, Kaigui, E-mail: kgzhu@buaa.edu.cn

    2016-04-15

    This study aims to investigate the effect of Ar{sup 8+} ions pre-damage on the following He{sup 2+} irradiation behavior of polycrystalline tungsten. We compared the irradiation resistance performance against 60 keV He{sup 2+} ions of undamaged tungsten samples with that of pre-damaged samples which were preliminarily exposed to 800 keV Ar{sup 8+} ions at a fluence of 4 × 10{sup 19} ions m{sup −2}. The experimental results indicate that the helium blistering of tungsten could be effectively relieved by the Ar{sup 8+} ions pre-damage, while the retention of helium around low energy desorption sites in the pre-damaged tungsten was larger than that of the undamaged samples. A strong orientation dependence of blistering had been observed, with the blister occurred preferentially on the surface of grains with normal direction close to <111>. The Ar{sup 8+} ions irradiation-induced damage altered the morphology of helium bubbles in tungsten exposed to the following He{sup 2+} irradiation significantly. The intensity of helium release peaks at relatively low temperatures (<600 K) was enhanced due to Ar{sup 8+} ions pre-damage. - Highlights: • Helium blistering on the surface of W was effectively relieved by Ar{sup 8+} ions pre-damage. • Strong orientation dependence of blister formation was observed. • Low temperature helium release peaks were increased due to Ar{sup 8+} ions pre-damage.

  9. Ultrafast probing of ejection dynamics of Rydberg atoms and molecular fragments from electronically excited helium nanodroplets.

    Science.gov (United States)

    Bünermann, Oliver; Kornilov, Oleg; Haxton, Daniel J; Leone, Stephen R; Neumark, Daniel M; Gessner, Oliver

    2012-12-07

    The ejection dynamics of Rydberg atoms and molecular fragments from electronically excited helium nanodroplets are studied with time-resolved extreme ultraviolet ion imaging spectroscopy. At excitation energies of 23.6 ± 0.2 eV, Rydberg atoms in n = 3 and n = 4 states are ejected on different time scales and with significantly different kinetic energy distributions. Specifically, n = 3 Rydberg atoms are ejected with kinetic energies as high as 0.85 eV, but their appearance is delayed by approximately 200 fs. In contrast, n = 4 Rydberg atoms appear within the time resolution of the experiment with considerably lower kinetic energies. Major features in the Rydberg atom kinetic energy distributions for both principal quantum numbers can be described within a simple elastic scattering model of localized perturbed atomic Rydberg atoms that are expelled from the droplet due to their repulsive interaction with the surrounding helium bath. Time-dependent kinetic energy distributions of He(2) (+) and He(3) (+) ions are presented that support the formation of molecular ions in an indirect droplet ionization process and the ejection of neutral Rydberg dimers on a similar time scale as the n = 3 Rydberg atoms.

  10. Paramagnetic Attraction of Impurity-Helium Solids

    Science.gov (United States)

    Bernard, E. P.; Boltnev, R. E.; Khmelenko, V. V.; Lee, D. M.

    2003-01-01

    Impurity-helium solids are formed when a mixture of impurity and helium gases enters a volume of superfluid helium. Typical choices of impurity gas are hydrogen deuteride, deuterium, nitrogen, neon and argon, or a mixture of these. These solids consist of individual impurity atoms and molecules as well as clusters of impurity atoms and molecules covered with layers of solidified helium. The clusters have an imperfect crystalline structure and diameters ranging up to 90 angstroms, depending somewhat on the choice of impurity. Immediately following formation the clusters aggregate into loosely connected porous solids that are submerged in and completely permeated by the liquid helium. Im-He solids are extremely effective at stabilizing high concentrations of free radicals, which can be introduced by applying a high power RF dis- charge to the impurity gas mixture just before it strikes the super fluid helium. Average concentrations of 10(exp 19) nitrogen atoms/cc and 5 x 10(exp 18) deuterium atoms/cc can be achieved this way. It shows a typical sample formed from a mixture of atomic and molecular hydrogen and deuterium. It shows typical sample formed from atomic and molecular nitrogen. Much of the stability of Im-He solids is attributed to their very large surface area to volume ratio and their permeation by super fluid helium. Heat resulting from a chance meeting and recombination of free radicals is quickly dissipated by the super fluid helium instead of thermally promoting the diffusion of other nearby free radicals.

  11. Helium atom excitations by the GW and Bethe-Salpeter many-body formalism

    CERN Document Server

    Li, Jing; Duchemin, Ivan; Blase, Xavier; Olevano, Valerio

    2016-01-01

    Helium atom is the simplest many-body electronic system provided by nature. The exact solution to the Schr\\"odinger equation is known for helium ground and excited states, and represents a workbench for any many-body methodology. Here we check ab initio many-body GW approximation and Bethe-Salpeter equation (BSE) against helium exact solution. Starting from Hartree-Fock, we show that GW and BSE yield impressingly accurate results on excitation energies and oscillator strength. These findings suggest that the accuracy of BSE and GW approximations is not significantly limited by self-interaction and self-screening problems even in this few electron limit. We further discuss our results in comparison to those obtained by time-dependent density-functional theory.

  12. Laser spectroscopy of atoms in superfluid helium for the measurement of nuclear spins and electromagnetic moments of radioactive atoms

    Energy Technology Data Exchange (ETDEWEB)

    Fujita, T., E-mail: tomomi.fujita@riken.jp [Osaka University, Department of Physics (Japan); Furukawa, T. [Tokyo Metropolitan University, Department of Physics (Japan); Imamura, K.; Yang, X. F. [RIKEN Nishina Center (Japan); Hatakeyama, A. [Tokyo University of Agriculture and Technology, Department of Applied Physics (Japan); Kobayashi, T. [RIKEN Center for Advanced Photonics (Japan); Ueno, H. [RIKEN Nishina Center (Japan); Asahi, K. [Tokyo Institute of Technology, Department of Physics (Japan); Shimoda, T. [Osaka University, Department of Physics (Japan); Matsuo, Y. [Hosei University, Department of Advanced Sciences (Japan); Collaboration: OROCHI Collaboration

    2015-11-15

    A new laser spectroscopic method named “OROCHI (Optical RI-atom Observation in Condensed Helium as Ion catcher)” has been developed for deriving the nuclear spins and electromagnetic moments of low-yield exotic nuclei. In this method, we observe atomic Zeeman and hyperfine structures using laser-radio-frequency/microwave double-resonance spectroscopy. In our previous works, double-resonance spectroscopy was performed successfully with laser-sputtered stable atoms including non-alkali Au atoms as well as alkali Rb and Cs atoms. Following these works, measurements with {sup 84−87}Rb energetic ion beams were carried out in the RIKEN projectile fragment separator (RIPS). In this paper, we report the present status of OROCHI and discuss its feasibility, especially for low-yield nuclei such as unstable Au isotopes.

  13. Effect of 800 keV argon ions pre-damage on the helium blister formation of tungsten exposed to 60 keV helium ions

    Science.gov (United States)

    Chen, Zhe; Han, Wenjia; Yu, Jiangang; Zhu, Kaigui

    2016-04-01

    This study aims to investigate the effect of Ar8+ ions pre-damage on the following He2+ irradiation behavior of polycrystalline tungsten. We compared the irradiation resistance performance against 60 keV He2+ ions of undamaged tungsten samples with that of pre-damaged samples which were preliminarily exposed to 800 keV Ar8+ ions at a fluence of 4 × 1019 ions m-2. The experimental results indicate that the helium blistering of tungsten could be effectively relieved by the Ar8+ ions pre-damage, while the retention of helium around low energy desorption sites in the pre-damaged tungsten was larger than that of the undamaged samples. A strong orientation dependence of blistering had been observed, with the blister occurred preferentially on the surface of grains with normal direction close to . The Ar8+ ions irradiation-induced damage altered the morphology of helium bubbles in tungsten exposed to the following He2+ irradiation significantly. The intensity of helium release peaks at relatively low temperatures (<600 K) was enhanced due to Ar8+ ions pre-damage.

  14. Controlled Reactions between Ultracold Alkali and Metastable Helium Atoms

    CERN Document Server

    Flores, Adonis Silva; Knoop, Steven

    2016-01-01

    In an ultracold, optically trapped mixture of $^{87}$Rb and metastable triplet $^4$He atoms we have studied trap loss for different spin-state combinations, for which interspecies Penning ionization is the main two-body loss process. We observe long trapping lifetimes for the purely quartet spin-state combination, indicating strong suppression of Penning ionization loss by at least two orders of magnitude. For the other spin-mixtures we observe short lifetimes that depend linearly on the doublet character of the entrance channel. We compare the extracted loss rate coefficient with recent predictions of multichannel quantum-defect theory for reactive collisions involving a strong exothermic loss channel and find near-universal loss for doublet scattering. Our work demonstrates control of reactive collisions by internal atomic state preparation, which also implies magnetic field tunability.

  15. Electron-phonon coupling and surface Debye temperature of Bi2Te3(111) from helium atom scattering

    DEFF Research Database (Denmark)

    Tamtogl, Anton; Kraus, Patrick; Avidor, Nadav

    2017-01-01

    We have studied the topological insulator Bi2Te3(111) by means of helium atom scattering. The average electron-phonon coupling lambda of Bi2Te3(111) is determined by adapting a recently developed quantum-theoretical derivation of the helium scattering probabilities to the case of degenerate...

  16. Optical and electron spin resonance studies of xenon-nitrogen-helium condensates containing nitrogen and oxygen atoms.

    Science.gov (United States)

    Boltnev, Roman E; Bykhalo, Igor B; Krushinskaya, Irina N; Pelmenev, Alexander A; Khmelenko, Vladimir V; Mao, Shun; Meraki, Adil; Wilde, Scott C; McColgan, Patrick T; Lee, David M

    2015-03-19

    We present the first observations of excimer XeO* molecules in molecular nitrogen films surrounding xenon cores of nanoclusters. Multishell nanoclusters form upon the fast cooling of a helium jet containing small admixtures of nitrogen and xenon by cold helium vapor (T = 1.5 K). Such nanoclusters injected into superfluid helium aggregate into porous impurity-helium condensates. Passage of helium gas with admixtures through a radio frequency discharge allows the storage of high densities of radicals stabilized in impurity-helium condensates. Intense recombination of the radicals occurs during destruction of such condensates and generates excited species observable because of optical emission. Rich spectra of xenon-oxygen complexes have been detected upon destruction of xenon-nitrogen-helium condensates. A xenon environment quenches metastable N((2)D) atoms but has a much weaker effect on the luminescence of N((2)P) atoms. Electron spin resonance spectra of N((4)S) atoms trapped in xenon-nitrogen-helium condensates have been studied. High local concentrations of nitrogen atoms (up to 10(21) cm(-3)) stabilized in xenon-nitrogen nanoclusters have been revealed.

  17. Creation evidence of the second non-dispersive Zakharenko wave by helium atomic beams in superfluid helium-II at low temperatures

    Indian Academy of Sciences (India)

    A A Zakharenko

    2007-10-01

    In this work, the experimental results of the creation of the second non-dispersive Zakharenko wave (ph = g ≠ 0) in the negative roton branch (the so-called second sound) of the bulk elementary excitations (BEEs) energy spectra are introduced. Several BEE signals detected by a bolometer situated in the isotopically pure liquid helium-II at low temperatures ∼ 100 mK are shown, which give evidence of negative roton creation in the liquid by helium atomic beams striking the liquid surface. The negative roton signals were clearly distinguished by the following ways: the negative roton signal created by helium atomic beams appeared earlier than the positive roton signal created by the beams, and presence of both positive and negative roton signals together. It is natural that the negative roton creation by the beams requires the 4He-atom energies ∼ 12 K, while the positive roton creation by the atomic beams requires energies ∼ 35 K. Therefore, successive increase in the heater power resulting in an increase in the 4He-atom energies gives solid evidence that the negative rotons are first created in the liquid by the helium atomic beams.

  18. Desorption Dynamics of Heavy Alkali Metal Atoms (Rb, Cs) off the Surface of Helium Nanodroplets

    CERN Document Server

    von Vangerow, J; Stienkemeier, F; Mudrich, M; Leal, A; Mateo, D; Hernando, A; Barranco, M; Pi, M

    2014-01-01

    We present a combined ion imaging and density functional theory study of the dynamics of the desorption process of rubidium and cesium atoms off the surface of helium nanodroplets upon excitation of the perturbed $6s$ and $7s$ states, respectively. Both experimental and theoretical results are well represented by the pseudodiatomic model for effective masses of the helium droplet in the desorption reaction of m_eff/m_He~10 (Rb) and 13 (Cs). Deviations from this model are found for Rb excited to the 6p state. Photoelectron spectra indicate that the dopant-droplet interaction induces relaxation into low-lying electronic states of the desorbed atoms in the course of the ejection process.

  19. Performance of Hyperspherical Harmonic Expansionon the Low-lying Pand D States of Helium Atom

    Institute of Scientific and Technical Information of China (English)

    2000-01-01

    The wave functions of the n 1,3P (n=2,3,4) and the n 1,3D (n=3,4,5) low-lying states ofthe helium atom are expanded into the complete sets of the symmetrically adapted basis functionsfrom hyperspherical harmonic functions in the angle part and of generalized Laguerre functions inthe radial part respectively, and are then augmented by the simplest type of Jastrow correlationfactor to incorporate electron-nucleus cusp only. The excellent agreement between the presentnonrelativistic eigen-energies and those from the sophisticated configuration interaction (CI)method for the examined states indicates that the hyperspherical harmonic method can also be applied to the P and the D excited states of the helium atom.

  20. Desorption dynamics of heavy alkali metal atoms (Rb, Cs) off the surface of helium nanodroplets.

    Science.gov (United States)

    von Vangerow, J; Sieg, A; Stienkemeier, F; Mudrich, M; Leal, A; Mateo, D; Hernando, A; Barranco, M; Pi, M

    2014-08-21

    We present a combined ion imaging and density functional theory study of the dynamics of the desorption process of rubidium and cesium atoms off the surface of helium nanodroplets upon excitation of the perturbed 6s and 7s states, respectively. Both experimental and theoretical results are well represented by the pseudodiatomic model for effective masses of the helium droplet in the desorption reaction of meff/mHe ≈ 10 (Rb) and 13 (Cs). Deviations from this model are found for Rb excited to the 6p state. Photoelectron spectra indicate that the dopant-droplet interaction induces relaxation into low-lying electronic states of the desorbed atoms in the course of the ejection process.

  1. Calculation of inelastic helium atom scattering from H2/ NaCl(001)

    DEFF Research Database (Denmark)

    Bruch, L.W.; Hansen, Flemming Yssing; Traeger, F.

    2011-01-01

    The one-phonon inelastic low energy helium atom scattering theory is adapted to cases where the target monolayer is a p(1 × 1) commensurate square lattice. Experimental data for para-H2/NaCl(001) are re-analyzed and the relative intensities of energy loss peaks in the range 6 to 9 meV are determi......The one-phonon inelastic low energy helium atom scattering theory is adapted to cases where the target monolayer is a p(1 × 1) commensurate square lattice. Experimental data for para-H2/NaCl(001) are re-analyzed and the relative intensities of energy loss peaks in the range 6 to 9 me...

  2. Continuous Compressed Sensing for Surface Dynamical Processes with Helium Atom Scattering

    Science.gov (United States)

    Jones, Alex; Tamtögl, Anton; Calvo-Almazán, Irene; Hansen, Anders

    2016-06-01

    Compressed Sensing (CS) techniques are used to measure and reconstruct surface dynamical processes with a helium spin-echo spectrometer for the first time. Helium atom scattering is a well established method for examining the surface structure and dynamics of materials at atomic sized resolution and the spin-echo technique opens up the possibility of compressing the data acquisition process. CS methods demonstrating the compressibility of spin-echo spectra are presented for several measurements. Recent developments on structured multilevel sampling that are empirically and theoretically shown to substantially improve upon the state of the art CS techniques are implemented. In addition, wavelet based CS approximations, founded on a new continuous CS approach, are used to construct continuous spectra. In order to measure both surface diffusion and surface phonons, which appear usually on different energy scales, standard CS techniques are not sufficient. However, the new continuous CS wavelet approach allows simultaneous analysis of surface phonons and molecular diffusion while reducing acquisition times substantially. The developed methodology is not exclusive to Helium atom scattering and can also be applied to other scattering frameworks such as neutron spin-echo and Raman spectroscopy.

  3. Study of helium and beryllium atoms with strong and short laser field; Etude des atomes d'helium et de beryllium en champ laser intense et bref

    Energy Technology Data Exchange (ETDEWEB)

    Laulan, St

    2004-09-01

    We present a theoretical study of the interaction between a two-active electron atom and an intense (10{sup 14} to 10{sup 15} W/cm{sup 2}) and ultrashort (from a few 10{sup -15} to a few 10{sup -18} s) laser field. In the first part, we describe the current experimental techniques able to produce a coherent radiation of high power in the UV-XUV regime and with femtosecond time duration. A theoretical model of a laser pulse is defined with such characteristics. Then, we develop a numerical approach based on B-spline functions to describe the atomic structure of the two-active electron system. A spectral non perturbative method is proposed to solve the time dependent Schroedinger equation. We focalize our attention on the description of the atomic double continuum states. Finally, we expose results on the double ionization of helium and beryllium atoms with intense and short laser field. In particular, we present total cross section calculations and ejected electron energy distributions in the double continuum after one- and two-photon absorption. (author)

  4. Absolute number densities of helium metastable atoms determined by atomic absorption spectroscopy in helium plasma-based discharges used as ambient desorption/ionization sources for mass spectrometry

    Science.gov (United States)

    Reininger, Charlotte; Woodfield, Kellie; Keelor, Joel D.; Kaylor, Adam; Fernández, Facundo M.; Farnsworth, Paul B.

    2014-10-01

    The absolute number densities of helium atoms in the 2s 3S1 metastable state were determined in four plasma-based ambient desorption/ionization sources by atomic absorption spectroscopy. The plasmas included a high-frequency dielectric barrier discharge (HF-DBD), a low temperature plasma (LTP), and two atmospheric-pressure glow discharges, one with AC excitation and the other with DC excitation. Peak densities in the luminous plumes downstream from the discharge capillaries of the HF-DBD and the LTP were 1.39 × 1012 cm- 3 and 0.011 × 1012 cm- 3, respectively. Neither glow discharge produced a visible afterglow, and no metastable atoms were detected downstream from the capillary exits. However, densities of 0.58 × 1012 cm- 3 and 0.97 × 1012 cm- 3 were measured in the interelectrode regions of the AC and DC glow discharges, respectively. Time-resolved measurements of metastable atom densities revealed significant random variations in the timing of pulsed absorption signals with respect to the voltage waveforms applied to the discharges.

  5. Metastable argon atom density in complex argon/acetylene plasmas determined by means of optical absorption and emission spectroscopy

    Science.gov (United States)

    Sushkov, Vladimir; Herrendorf, Ann-Pierra; Hippler, Rainer

    2016-10-01

    Optical emission and absorption spectroscopy has been utilized to investigate the instability of acetylene-containing dusty plasmas induced by growing nano-particles. The density of Ar(1s5) metastable atoms was derived by two methods: tunable diode laser absorption spectroscopy and with the help of the branching ratio method of emitted spectral lines. Results of the two techniques agree well with each other. The density of Ar(1s3) metastable atoms was also measured by means of optical emission spectroscopy. The observed growth instability leads to pronounced temporal variations of the metastable and other excited state densities. An analysis of optical line ratios provides evidence for a depletion of free electrons during the growth cycle but no indication for electron temperature variations.

  6. Measurement of helium-like and hydrogen-like argon spectra using double-crystal X-ray spectrometers on EAST

    Science.gov (United States)

    Lyu, B.; Chen, J.; Hu, R. J.; Wang, F. D.; Li, Y. Y.; Fu, J.; Shen, Y. C.; Bitter, M.; Hill, K. W.; Delgado-Aparicio, L. F.; Pablant, N.; Lee, S. G.; Ye, M. Y.; Shi, Y. J.; Wan, B. N.

    2016-11-01

    A two-crystal assembly was deployed on the tangential X-ray crystal spectrometer to measure both helium-like and hydrogen-like spectra on EAST. High-quality helium-like and hydrogen-like spectra were observed simultaneously for the first time on one detector for a wide range of plasma parameters. Profiles of line-integrated core ion temperatures inferred from two spectra were consistent. Since tungsten was adopted as the upper divertor material, one tungsten line (W XLIV at 4.017 Å) on the short-wavelength side of the Lyman-α line (Lα1) was identified for typical USN discharges, which was diffracted by a He-like crystal (2d = 4.913 Å). Another possible Fe XXV line (1.85 Å) was observed to be located on the long-wavelength side of resonance line (w), which was diffracted from a H-like crystal (2d = 4.5622 Å) on the second order. Be-like argon lines were also observable that fill the detector space between the He-like and H-like spectra.

  7. Helium-argon isotopic tracing for the Pb-Zn-Ag polymetallic ore deposits in the central-south segment of the Da Hinggan Ling Range

    Institute of Scientific and Technical Information of China (English)

    WANG Baode; NIU Shuyin; SUN Aiqun; HU Huabin; LIU Yaming; GUO Lijun; WANG Shuo

    2008-01-01

    In recent years big strides have been made in the exploration of ores in the central-south segment of the Da Hinggan Ling Range, though some debates still exist on the metallogenesis and sources of ore-forming materials.Pyrite and other sulfides in direct relation to the Pb-Zn-Ag ore deposits were chosen for the He and Ar isotopic analysis of ore-forming fluids, and the first He and Ar isotope data have been obtained from the study region.3He/4He ratios in 14 samples collected from 7 mining districts are 2.17x10-6-12.52×10-6, averaging 6.86×10-6 and their R/Ra ratios are 1.56-9.01 Ra, averaging 4.37 Ra. By projecting the data points onto the 3He-4He concentrations diagram, all the points fall near the mantle helium area. The calculated mantle-source helium ratios are within the range of 19.58%-76.96%, with an average of 49.52%. Argon isotopic characteristics are close to those of mantle source, indicating that the ore-forming material was transport upwards via the multi-stage evolution of mantle plume and concentrated as ores in the favorable loci of mantle branch structures.

  8. Measurement of the hyperfine splitting of {sup 133}Cs atoms in superfluid helium

    Energy Technology Data Exchange (ETDEWEB)

    Imamura, K., E-mail: kimamura@riken.jp [RIKEN Nishina Center (Japan); Furukawa, T. [Tokyo Metropolitan University, Department of Physics (Japan); Yang, X. F. [Peking University, School of Physics (China); Mitsuya, Y. [Meiji University, Department of Physics (Japan); Fujita, T. [Osaka University, Department of Physics (Japan); Hayasaka, M. [Tokyo Gakugei University, Department of Physics (Japan); Kobayashi, T. [RIKEN Center for Advanced Photonics (Japan); Hatakeyama, A. [Tokyo University of Agriculture and Technology, Department of Applied Physics (Japan); Ueno, H. [RIKEN Nishina Center (Japan); Odashima, H. [Meiji University, Department of Physics (Japan); Matsuo, Y. [Hosei University, Department of Advanced Sciences (Japan)

    2015-04-15

    We have been developing a new nuclear laser spectroscopy method named “OROCHI” (Optical RI-atom Observation in Condensed Helium as Ion-catcher). OROCHI utilizes superfluid helium (He II) not only as an efficient stopping medium of highly energetic ions but also as a host matrix of in-situ atomic laser spectroscopy. Using these characteristic of He II, we produce atomic spin polarization and measure Zeeman and hyperfine structure (HFS) splitting using laser-RF (radio frequency) / MW (microwave) double resonance method. From the measured energy splittings, we can deduce nuclear spins and moments. So far, we have conducted a series of experiments using both stable ({sup 85,87}Rb, {sup 133}Cs, {sup 197}Au, {sup 107,109}Ag) and unstable isotopes ({sup 84,86}Rb) to confirm the feasibility of OROCHI method, especially observing Zeeman resonance and determining nuclear spins. The measurement of HFS splitting of atoms introduced into He II is indispensable to clarify the nuclear properties by deducing nuclear moments as well as the study of nuclear spins. For this purpose, we perform a precision measurement of HFS of {sup 133}Cs atoms immersed in He II using laser ablation technique. In this paper, we describe the result of the experiment.

  9. Influence of Helium Atoms Absorption on the Emission Properties of Carbon Nanotubes

    Science.gov (United States)

    Umaev, S. M.; Levchenko, A. A.; Kolesnikov, N. N.; Filatov, S. V.

    2017-04-01

    We investigated the emission properties of charge sources based on carbon nanotubes prepared by arc discharge deposition of nanotubes onto a flat copper substrate (Borisenko et al. in Instrum Exp Tech 57(6):755, 2014; Low Temp Phys 41(7):567, 2015). The charge sources were submerged into superfluid helium at temperature T=1.3 K. The collector fixed above the charge source at a distance of 0.3 mm was connected to an electrometer. The current of charges was measured by the electrometer when a high voltage was applied to the charge source. In the originally prepared source, the emission of charges (electrons) on the level of 10^{-10}A is observed at a negative voltage above U=80 V and increases with increasing voltage. If the source of charge was kept in liquid helium for 15 h, the current-voltage characteristic changed significantly. The current of charges on the same level of 10^{-10} A was registered at a voltage of U=150 V. Extraction of gases from the source placed in a vacuum chamber at room temperature for 48 h leads to the complete recovery of the emission properties. One can assume that the degradation of the emission properties of the sources is associated with the adsorption of helium atoms by carbon nanotubes at low temperatures. We did not observe any degradation of the emission properties of the charge sources in the case of positive charges injection into superfluid helium.

  10. Formation of bimetallic clusters in superfluid helium nanodroplets analysed by atomic resolution electron tomography

    Science.gov (United States)

    Haberfehlner, Georg; Thaler, Philipp; Knez, Daniel; Volk, Alexander; Hofer, Ferdinand; Ernst, Wolfgang E.; Kothleitner, Gerald

    2015-10-01

    Structure, shape and composition are the basic parameters responsible for properties of nanoscale materials, distinguishing them from their bulk counterparts. To reveal these in three dimensions at the nanoscale, electron tomography is a powerful tool. Advancing electron tomography to atomic resolution in an aberration-corrected transmission electron microscope remains challenging and has been demonstrated only a few times using strong constraints or extensive filtering. Here we demonstrate atomic resolution electron tomography on silver/gold core/shell nanoclusters grown in superfluid helium nanodroplets. We reveal morphology and composition of a cluster identifying gold- and silver-rich regions in three dimensions and we estimate atomic positions without using any prior information and with minimal filtering. The ability to get full three-dimensional information down to the atomic scale allows understanding the growth and deposition process of the nanoclusters and demonstrates an approach that may be generally applicable to all types of nanoscale materials.

  11. Atomic collisions in suprafluid helium-nanodroplets: timescales for metal-cluster formation derived from He-density functional theory.

    Science.gov (United States)

    Hauser, Andreas W; Volk, Alexander; Thaler, Philipp; Ernst, Wolfgang E

    2015-04-28

    Collision times for the coinage metal atoms Cu, Ag and Au in He-droplets are derived from helium density functional theory and molecular dynamics simulations. The strength of the attractive interaction between the metal atoms turns out to be less important than the mass of the propagating metal atoms. Even for small droplets consisting of a few thousand helium atoms, the collision times are shortest for Cu, followed by Ag and Au, despite the higher binding energy of Au2 compared to Cu2.

  12. Bibliography of electron and photon cross sections with atoms and molecules published in the 20th century. Argon

    Energy Technology Data Exchange (ETDEWEB)

    Hayashi, Makoto [Gaseous Electronics Institute, Nagoya, Aichi (Japan)

    2003-01-01

    A bibliography of original and review reports of experiments or theories of electron and photon cross sections and also electron swarm data are presented for atomic or molecular species with specified targets. These works covered 17 atoms and 51 molecules. The present bibliography is only for argon (Ar). About 1,960 papers were compiled. A comprehensive author index is included. The bibliography covers the period 1921 through 2000 for Ar. Finally, author's recommended Ar electron collision cross section set is given in numerical tables. (author)

  13. Magnetic Dichroism of Potassium Atoms on the Surface of Helium Nanodroplets

    Science.gov (United States)

    Nagl, Johann; Auböck, Gerald; Callegari, Carlo; Ernst, Wolfgang E.

    2007-02-01

    The population ratio of Zeeman sublevels of atoms on the surface of superfluid helium droplets (T=0.37K) has been measured. Laser induced fluorescence spectra of K atoms are measured in the presence of a moderately strong magnetic field (2.9 kG). The relative difference between the two states of circular polarization of the exciting laser is used to determine the electron spin polarization of the ensemble. Equal fluorescence levels indicate that the two spin sublevels of the ground-state K atom are equipopulated, within 1%. Thermalization to 0.37 K would give a population ratio of 0.35. We deduce that the rate of spin relaxation induced by the droplet must be <520/s. For the K2 triplet dimer we find instead full thermalization of the spin.

  14. Diffraction of helium atom beams from a micro-structured reflection grating

    Energy Technology Data Exchange (ETDEWEB)

    Zhao, Bum Suk; Meijer, Gerard; Schoellkopf, Wieland [Fritz-Haber-Institut der Max-Planck-Gesellschaft, Berlin (Germany); Schulz, Stephan [Universitaet Ulm (Germany). Institut fuer Quanteninformationsverarbeitung

    2008-07-01

    We have observed high-resolution diffraction patterns of a thermal-energy helium-atom beam reflected from a micro-structured surface grating at grazing incidence. The grating has a periodicity of 20 {mu}m and consists of 10-{mu}m-wide Cr stripes patterned on a quartz substrate. Fully-resolved diffraction peaks up to the 7-th order are observed at grazing incidence angles up to 20 mrad. With changes in de Broglie wavelength or incidence angle the relative diffraction intensities show significant variations which are attributed to the atom-surface Casimir-van der Waals potential. In addition, the overall probability of coherent reflection is found to increase with increasing de Broglie wavelength and decreasing incidence angle. We discuss whether this behavior indicates quantum reflection at the long-range attractive branch of the atom-surface potential.

  15. Gas temperature determination in an argon non-thermal plasma at atmospheric pressure from broadenings of atomic emission lines

    Science.gov (United States)

    Yubero, C.; Rodero, A.; Dimitrijevic, M. S.; Gamero, A.; García, M. C.

    2017-03-01

    In this work a new spectroscopic method, allowing gas temperature determination in argon non-thermal plasmas sustained at atmospheric pressure, is presented. The method is based on the measurements of selected pairs of argon atomic lines (Ar I 603.2 nm/Ar I 549.6 nm, Ar I 603.2 nm/Ar I 522.1 nm, Ar I 549.6 nm/Ar I 522.1 nm). For gas temperature determination using the proposed method, there is no need of knowing the electron density, neither making assumptions on the degree of thermodynamic equilibrium existing in the plasma. The values of the temperatures obtained using this method, have been compared with the rotational temperatures derived from the OH ro-vibrational bands, using both, the well-known Boltzmann-plot technique and the best fitting to simulated ro-vibrational bands. A very good agreement has been found.

  16. Energetic neutral helium atoms as a tool to study the heliosphere and the local interstellar medium

    Science.gov (United States)

    Swaczyna, Pawel; Grzedzielski, Stan; Bzowski, Maciej

    2015-04-01

    The aim of our study is to determine the utility of helium energetic neutral atoms (ENA) in the studies of the outer heliosphere, its boundary region, and the nearby interstellar medium, and to assess the requirements for future instruments to enable them to observe He ENA fluxes. Presently, studying these regions is rendered possible mostly by combining the in-situ measurements by the plasma and cosmic-ray instruments on Voyagers and the remote-sensing observations of H ENA from IBEX. Helium as the second most abundant species in the universe could potentially enable further extension of our knowledge about nearest surroundings of the Sun. We assessed the expected emission of the heliospheric He ENA and of He ENA from the nearby interstellar medium. To estimate the heliospheric emission of He ENA we used a simple model of the heliosphere and performed numerical simulations to determine the distribution of various populations of helium ions in the inner heliosphere. Based on this model, we calculated fluxes of He ENA created by charge exchange between helium ions and neutral atoms over a wide energy range from 0.5 keV/nuc up to 1 MeV/nuc. We included binary interactions between various combinations of hydrogen and helium ions and atoms. We also included the signal from the vicinity of the heliosphere produced via the secondary ENA mechanism, which is most likely the source for the observed IBEX Ribbon. The mean free path against ionization of He ENA in the local interstellar medium reaches about 8000 AU for atoms with an energy of a few keV. This is about 10 times more than the mean free path against ionization for hydrogen atoms at the same energy. Thus emission of helium ENA from hypothetic extraheliospheric sources could be detectable from larger distances than the hydrogen atoms. This could provide a novel method of sounding the sources of suprathermal ions that might operate in the surrounding of the heliosphere. The He ENA produced by charge-exchange could

  17. On the theory of (e, 2e) reactions in atomic hydrogen and helium

    Science.gov (United States)

    Byron, F. W.; Joachain, C. J.; Piraux, B.

    1984-12-01

    We compare the results of eikonal-Born series calculations which we have performed for the (e, 2e) reaction in atomic hydrogen with recent absolute measurements of triple differential cross sections for that process, carried out in the asymmetric coplanar geometry. We find that second-order effects play a crucial role in understanding both the angular positions and the magnitudes of the binary and recoil peaks. The implications of our analysis for the case of (e, 2e) reactions in helium are also discussed.

  18. Scaled-energy spectroscopy of helium \\|M\\|=1 Rydberg atoms in a static electric field

    Science.gov (United States)

    Kips, Annemieke; Vassen, Wim; Hogervorst, Wim; Dando, Paul A.

    1998-10-01

    We present scaled-energy spectra on helium Rydberg atoms in a static electric field. \\|M\\|=1 states were studied in excitation from the 2 1S0 metastable state. Spectra were recorded for ɛ=-2.940(4), ɛ=-2.350(4), both below the saddle point, and ɛ=-1.760(4), above the saddle point. Closed-orbit theory was applied to interpret the spectra. A recent extension to closed-orbit theory, incorporating core effects, was used. This significantly improved agreement between experiment and theory.

  19. Time-resolved studies on the collapse of magnesium atom foam in helium nanodroplets

    CERN Document Server

    Göde, S; Tiggesbäumker, J; Meiwes-Broer, K -H

    2012-01-01

    Magnesium atoms embedded in superfluid helium nanodroplets have been identified to arrange themselves in a metastable network, refered to as foam. In order to investigate the ionization dynamics of this unique structure with respect to a possible light-induced collapse the femtosecond dual-pulse spectroscopy technique is applied. Around zero optical delay a strong feature is obtained which represents a direct probe of the foam response. We found that upon collapse, ionization is reduced. A particlar intensity ratio of the pulses allows to address either direct ionization or photoactivation of the neutral complexes, thus affecting reaction pathways. A simplified excitation scheme visualizes possible scenarios in accordance with the experimental observations.

  20. Effects of impurity molecules on the lifetime of antiprotonic helium atoms

    CERN Document Server

    Juhász, B; Hayano, R S; Hori, Masaki; Horváth, D; Ishikawa, T; Torii, H A; Widmann, E; Yamaguchi, H; Yamazaki, T

    2004-01-01

    Quenching of metastable antiprotonic helium atoms in collisions with hydrogen and deuterium molecules has been studied using laser spectroscopy at CERN's antiproton decelerator. The temperature dependence of the quenching cross sections of the antiprotonic states (n, l) = (37, 34), (38, 35) and (38, 37) has been investigated and a deviation from the Arrhenius law was found at low temperatures. In case of the state (38, 37) with deuterium, detailed measurements revealed that the quenching cross section levels off at low temperatures indicating a strong quantum tunneling effect. (14 refs).

  1. Observation of dynamic atom-atom correlation in liquid helium in real space.

    Science.gov (United States)

    Dmowski, W; Diallo, S O; Lokshin, K; Ehlers, G; Ferré, G; Boronat, J; Egami, T

    2017-05-04

    Liquid (4)He becomes superfluid and flows without resistance below temperature 2.17 K. Superfluidity has been a subject of intense studies and notable advances were made in elucidating the phenomenon by experiment and theory. Nevertheless, details of the microscopic state, including dynamic atom-atom correlations in the superfluid state, are not fully understood. Here using a technique of neutron dynamic pair-density function (DPDF) analysis we show that (4)He atoms in the Bose-Einstein condensate have environment significantly different from uncondensed atoms, with the interatomic distance larger than the average by about 10%, whereas the average structure changes little through the superfluid transition. DPDF peak not seen in the snap-shot pair-density function is found at 2.3 Å, and is interpreted in terms of atomic tunnelling. The real space picture of dynamic atom-atom correlations presented here reveal characteristics of atomic dynamics not recognized so far, compelling yet another look at the phenomenon.

  2. Analysis of tungsten carbide coatings by infrared laser-induced argon spark with inductively coupled plasma atomic emission spectrometry

    Science.gov (United States)

    Kanický, V.; Otruba, V.; Mermet, J.-M.

    2000-10-01

    Infrared laser ablation was studied for application to the analysis of plasma-sprayed tungsten carbide/cobalt coatings. The potential of the laser induced argon-spark (LINA-Spark™), as a sample introduction device in inductively coupled plasma atomic emission spectrometry was studied. The use of an IR laser along with defocusing led to laser-induced microplasma-based ablation. The mass ablation rate, represented by the ICP emission intensity per laser beam unit area, exhibited a flat increase in the irradiance range 2-250 GW/cm 2. A low slope (0.5) of this dependence in log-log scale gave evidence of plasma shielding. The steep increase in the measured acoustic signal when focused in front of the sample, i.e. in argon, indicated a breakdown of argon. Consequently, considerably lower ICP emissions were observed within the same range of irradiance. The cobalt/tungsten line intensity ratio in the ICP was practically constant from 1.5 up to at least 250 GW/cm 2. Acceptable precision (R.S.D.<5%) was obtained without internal standardization for irradiance between 2 and 8 GW/cm 2. Optimization of the laser pulse energy, repetition rate, beam focusing and sample displacement during interaction led to the linearization of dependences of signal vs. cobalt percentage, at least up to the highest studied value of 23% Co.

  3. Communication: Angular momentum alignment and fluorescence polarization of alkali atoms photodetached from helium nanodroplets

    Energy Technology Data Exchange (ETDEWEB)

    Hernando, Alberto; Beswick, J. Alberto; Halberstadt, Nadine [LCAR-IRSAMC, Université Toulouse 3 - Paul Sabatier and CNRS, 31062 Toulouse (France)

    2013-12-14

    The theory of photofragments angular momentum polarization is applied to the photodetachment of an electronically excited alkali atom from a helium nanocluster (N = 200). The alignment of the electronic angular momentum of the bare excited alkali atoms produced is calculated quantum mechanically by solving the excited states coupled equations with potentials determined by density functional theory (DFT). Pronounced oscillations as a function of excitation energy are predicted for the case of Na@(He){sub 200}, in marked contrast with the absorption cross-section and angular distribution of the ejected atoms which are smooth functions of the energy. These oscillations are due to quantum interference between different coherently excited photodetachment pathways. Experimentally, these oscillations should be reflected in the fluorescence polarization and polarization-resolved photoelectron yield of the ejected atoms, which are proportional to the electronic angular momentum alignment. In addition, this result is much more general than the test case of NaHe{sub 200} studied here. It should be observable for larger droplets, for higher excited electronic states, and for other alkali as well as for alkali-earth atoms. Detection of these oscillations would show that the widely used pseudo-diatomic model can be valid beyond the prediction of absorption spectra and could help in interpreting parts of the dynamics, as already hinted by some experimental results on angular anisotropy of bare alkali fragments.

  4. Communication: angular momentum alignment and fluorescence polarization of alkali atoms photodetached from helium nanodroplets.

    Science.gov (United States)

    Hernando, Alberto; Beswick, J Alberto; Halberstadt, Nadine

    2013-12-14

    The theory of photofragments angular momentum polarization is applied to the photodetachment of an electronically excited alkali atom from a helium nanocluster (N = 200). The alignment of the electronic angular momentum of the bare excited alkali atoms produced is calculated quantum mechanically by solving the excited states coupled equations with potentials determined by density functional theory (DFT). Pronounced oscillations as a function of excitation energy are predicted for the case of Na@(He)200, in marked contrast with the absorption cross-section and angular distribution of the ejected atoms which are smooth functions of the energy. These oscillations are due to quantum interference between different coherently excited photodetachment pathways. Experimentally, these oscillations should be reflected in the fluorescence polarization and polarization-resolved photoelectron yield of the ejected atoms, which are proportional to the electronic angular momentum alignment. In addition, this result is much more general than the test case of NaHe200 studied here. It should be observable for larger droplets, for higher excited electronic states, and for other alkali as well as for alkali-earth atoms. Detection of these oscillations would show that the widely used pseudo-diatomic model can be valid beyond the prediction of absorption spectra and could help in interpreting parts of the dynamics, as already hinted by some experimental results on angular anisotropy of bare alkali fragments.

  5. GASP - THERMODYNAMIC AND TRANSPORT PROPERTIES OF HELIUM, METHANE, NEON, NITROGEN, CARBON MONOXIDE, CARBON DIOXIDE, OXYGEN, AND ARGON

    Science.gov (United States)

    Hendricks, R. C.

    1994-01-01

    A computer program, GASP, has been written to calculate the thermodynamic and transport properties of argon, carbon dioxide, carbon monoxide, fluorine, methane, neon, nitrogen, and oxygen. GASP accepts any two of pressure, temperature, or density as input. In addition, entropy and enthalpy are possible inputs. Outputs are temperature, density, pressure, entropy, enthalpy, specific heats, expansion coefficient, sonic velocity, viscosity, thermal conductivity, and surface tension. A special technique is provided to estimate the thermal conductivity near the thermodynamic critical point. GASP is a group of FORTRAN subroutines. The user typically would write a main program that invoked GASP to provide only the described outputs. Subroutines are structured so that the user may call only those subroutines needed for his particular calculations. Allowable pressures range from 0.l atmosphere to 100 to l,000 atmospheres, depending on the fluid. Similarly, allowable pressures range from the triple point of each substance to 300 degrees K to 2000 degrees K, depending on the substance. The GASP package was developed to be used with heat transfer and fluid flow applications. It is particularly useful in applications of cryogenic fluids. Some problems associated with the liquefication, storage, and gasification of liquefied natural gas and liquefied petroleum gas can also be studied using GASP. This program is written in FORTRAN IV for batch execution and is available for implementation on IBM 7000 series computers. GASP was developed in 1971.

  6. GASP - THERMODYNAMIC AND TRANSPORT PROPERTIES OF HELIUM, METHANE, NEON, NITROGEN, CARBON MONOXIDE, CARBON DIOXIDE, OXYGEN, AND ARGON

    Science.gov (United States)

    Hendricks, R. C.

    1994-01-01

    A computer program, GASP, has been written to calculate the thermodynamic and transport properties of argon, carbon dioxide, carbon monoxide, fluorine, methane, neon, nitrogen, and oxygen. GASP accepts any two of pressure, temperature, or density as input. In addition, entropy and enthalpy are possible inputs. Outputs are temperature, density, pressure, entropy, enthalpy, specific heats, expansion coefficient, sonic velocity, viscosity, thermal conductivity, and surface tension. A special technique is provided to estimate the thermal conductivity near the thermodynamic critical point. GASP is a group of FORTRAN subroutines. The user typically would write a main program that invoked GASP to provide only the described outputs. Subroutines are structured so that the user may call only those subroutines needed for his particular calculations. Allowable pressures range from 0.l atmosphere to 100 to l,000 atmospheres, depending on the fluid. Similarly, allowable pressures range from the triple point of each substance to 300 degrees K to 2000 degrees K, depending on the substance. The GASP package was developed to be used with heat transfer and fluid flow applications. It is particularly useful in applications of cryogenic fluids. Some problems associated with the liquefication, storage, and gasification of liquefied natural gas and liquefied petroleum gas can also be studied using GASP. This program is written in FORTRAN IV for batch execution and is available for implementation on IBM 7000 series computers. GASP was developed in 1971.

  7. Helium and Argon Isotopic Composition of Cenozoic Alkali Basalts and Mantle-Derived Xenoliths from Kuandian, Liaoning Province, China

    Institute of Scientific and Technical Information of China (English)

    吴茂炳; 王先彬; 叶先仁; 刘春燕

    2004-01-01

    The noble gas isotopic composition and content data of 2 alkali basalts, 3 lherzolite xenoliths and one clinopyroxene megacryst from the Kuandian region have confirmed the occurrence of a fractionation of noble gases during magmatism. Light noble gases such as He and Ne are high in mobility and appear to be incompatible as compared with heavy ones (such as Kr and Xe). Therefore, light noble gases are abundant in volcanics, especially in the volcanics with bubbles; lherzolite xenoliths have relatively high heavy noble gases. The clinopyroxene megacryst has the lowest abundance of noble gases, probably due to its high P-T origin. Noble gas isotopic composition of the clinopyroxene megacryst reveals that the mantle source beneath the Kuandian area has an MORB-like reservoir with 3He / 4He ratio of ~10 Ra (Ra: atmospheric 3He / 4He ratio) and 40 Ar/ 36 Ar ratio of 345.6 . The lherzolite xenoliths possess moderate 3He / 4He ratios of 2.59 - 4.53 Ra, reflecting the loss of primary helium during rock deformation or metasomatism caused by enriched mantle fluids during the up-lifting. The alkali volcanics have very low 3He / 4He ratios ( 0.47 - 0.61 Ra), indicating a contribution of radiogenic 4He , probably having resulted from crust contamination. Most of the samples have excess 21 Ne and 22 Ne as compared with atmospheric neon, but Kr and Xe isotopic compositions are indistinguishable from atmospheric values within uncertainties with only individual samples having excess 129 Xe , 134 Xe and 136 Xe .

  8. Interactions of satellite-speed helium atoms with satellite surfaces. III. Drag coefficients from spatial and energy distributions of reflected helium atoms. [1235-O and 6061 T-6 aluminum

    Energy Technology Data Exchange (ETDEWEB)

    Sharma, P.K.; Knuth, E.L.

    1977-12-01

    Spatial and energy distributions of helium atoms scattered from an anodized 1235-0 aluminum surface as well as the tangential and normal momentum accommodation coefficients calculated from these distributions are reported. A procedure for calculating drag coefficients from measured values of spatial and energy distributions is given. The drag coefficient calculated for a 6061 T-6 aluminum sphere is included.

  9. Isotope effect in collision between helium atom and hydrogen bromide molecule

    Institute of Scientific and Technical Information of China (English)

    Yu Chun-Ri; Cheng Xin-Lu; Yang Xiang-Dong

    2008-01-01

    The anisotropic potential developed in our previous research and the close-coupling method are applied to the HBr-3He(4He,5He,6He,7He)system,and the partial cross sections(PCSs)at the incident energy of 60 meV are calculated.Based on the calculations,the influences of the isotope helium atom on PCSs are discussed in detail.The results show that the excitation PCSs converge faster than the elastic PCSs for the collision energy and the systems considered here.Also the excitation PCSs converge more rapidly for the high-excited states.The tail effect is present only in elastic scattering and low-excited states but not in high-excited states.With the increase of reduced mass of the collision system,the converging speed of the elastic and excitation PCSs slows down,and the tail effect goes up.

  10. Single ionization of helium atoms by energetic fully stripped carbon ions

    Institute of Scientific and Technical Information of China (English)

    Ebrahim Ghanbari-Adivi; Sadjad Eskandari

    2015-01-01

    A four-body distorted wave approximation is presented for theoretical investigations of the single ionization of ground-state helium atoms by fully stripped carbon ions at impact energies of 2 MeV/amu and 100 MeV/amu. The nine-dimensional integrals for the partial quantum-mechanical transition amplitudes of the specified reaction are reduced to some analytical expressions or one-dimensional integrals over real variables. Fully differential cross sections (FDCSs) are calculated and compared with their experimental values as well as the results obtained from other theories. Despite the simplicity and quickness of the proposed quadrature, the comparison shows that the obtained results are in reasonable agreement with the experiment and are compatible with those of other complicated theories.

  11. Scaled-energy spectroscopy of helium vertical bar M vertical bar=1 Rydberg atoms in a static electric field

    NARCIS (Netherlands)

    Kips, A.; Vassen, W.; Hogervorst, W.; Dando, P.A.

    1998-01-01

    We present scaled-energy spectra on helium Rydberg atoms in a static electric field. /M/ = 1 states were studied in excitation from the 2 S-1(0) metastable state. Spectra were recorded for epsilon = -2.940(4), epsilon = -2.350(4), both below the saddle point, and epsilon = -1.760(4), above the saddl

  12. The ASACUSA experiment at CERN's AD antiproton decelerator catches antiprotons in helium, where the antiprotons replace electrons, giving exotics atoms.

    CERN Multimedia

    Loïez, P

    2000-01-01

    Photo 03: Laser beams are prepared for shooting at antiprotonic helium atoms. Left to right: Masaki Hori (Tokyo University) and John Eades (CERN). Photo 01: Dye laser triggered by "YAG" laser. Photo 02: Masaki Hori adjusting optical system of laser beams.

  13. Antiproton–to–electron mass ratio determined by two-photon laser spectroscopy of antiprotonic helium atoms

    Directory of Open Access Journals (Sweden)

    Sótér A.

    2014-03-01

    Full Text Available The ASACUSA collaboration of CERN has recently carried out two-photon laser spectroscopy of antiprotonic helium atoms. Three transition frequencies were determined with fractional precisions of 2.3–5 parts in 109. By comparing the results with three-body QED calculations, the antiproton-to-electron mass ratio was determined as 1836.1526736(23.

  14. Analysis of tree leaves, bark and wood by sequential inductively coupled argon plasma atomic emission spectrometry

    Science.gov (United States)

    Verbeek, A. A.

    The analysis of extracts from tree leaf, bark and wood samples for Ca, Mg, K, Na, P, Mn, Fe, Al, B, Cu and Zn by inductively coupled argon plasma sequential emission spectrometry is described. Recovery percentages for simulated tree extracts and for spiked tree samples are presented together with typical analysis values for a leaf and a wood sample. The choice of analytical line for each element is discussed and spectral interferences, not listed in the ICP tables of Boumans, of Cu on the 214.9 nm line of P and of Fe on the 249.7 nm line of B are noted.

  15. LIF measurements for validation of collisional-radiative modelling of atomic helium in the edge of a fusion plasma

    Energy Technology Data Exchange (ETDEWEB)

    Krychowiak, M; Koenig, R; Wolf, R; Klinger, T [Max-Planck-Institut fuer Plasmaphysik, EURATOM Association, Greifswald (Germany); Mertens, Ph; Schweer, B; Brezinsek, S; Schmitz, O; Samm, U [Institut fuer Energieforschung (Plasmaphysik), FZ Juelich, EURATOM Association, TEC, Juelich (Germany); Brix, M, E-mail: maciej.krychowiak@ipp.mpg.d [UKAEA, JET-Experimental Department, EURATOM Association, Culham Science Centre, Abingdon, Oxfordshire, OX14 3DB (United Kingdom)

    2010-05-01

    Local values of the electron density and temperature in the edge of a fusion plasma can be derived with high space and time resolution by the use of line radiation of atomic helium beams. The accuracy of this method is mainly limited by the uncertainties in the collisional-radiative (CR) model which is needed in order to obtain both plasma parameters from the measured relative intensities of atomic helium lines. Laser-induced fluorescence spectroscopy on a thermal helium beam in the edge plasma of the tokamak TEXTOR in Juelich was applied to validate the CR model of helium. By use of a high-power, pulsed laser system (a dye laser pumped by an excimer laser) several laser excitation schemes starting from the n=2 levels have been tried. The fluorescence light was observed at the laser wavelength and elsewhere in the spectrum providing information on population densities of initial levels as well as on collisional population transfer between excited levels. This paper summarises the results of the measurements, showing principal limits and possible improvements of this experimental validation method of the CR model of the diagnostic helium beam.

  16. LIF measurements for validation of collisional-radiative modelling of atomic helium in the edge of a fusion plasma

    Science.gov (United States)

    Krychowiak, M.; Mertens, Ph; König, R.; Schweer, B.; Brezinsek, S.; Schmitz, O.; Brix, M.; Samm, U.; Wolf, R.; Klinger, T.

    2010-05-01

    Local values of the electron density and temperature in the edge of a fusion plasma can be derived with high space and time resolution by the use of line radiation of atomic helium beams. The accuracy of this method is mainly limited by the uncertainties in the collisional-radiative (CR) model which is needed in order to obtain both plasma parameters from the measured relative intensities of atomic helium lines. Laser-induced fluorescence spectroscopy on a thermal helium beam in the edge plasma of the tokamak TEXTOR in Jülich was applied to validate the CR model of helium. By use of a high-power, pulsed laser system (a dye laser pumped by an excimer laser) several laser excitation schemes starting from the n=2 levels have been tried. The fluorescence light was observed at the laser wavelength and elsewhere in the spectrum providing information on population densities of initial levels as well as on collisional population transfer between excited levels. This paper summarises the results of the measurements, showing principal limits and possible improvements of this experimental validation method of the CR model of the diagnostic helium beam.

  17. GASP: A computer code for calculating the thermodynamic and transport properties for ten fluids: Parahydrogen, helium, neon, methane, nitrogen, carbon monoxide, oxygen, fluorine, argon, and carbon dioxide. [enthalpy, entropy, thermal conductivity, and specific heat

    Science.gov (United States)

    Hendricks, R. C.; Baron, A. K.; Peller, I. C.

    1975-01-01

    A FORTRAN IV subprogram called GASP is discussed which calculates the thermodynamic and transport properties for 10 pure fluids: parahydrogen, helium, neon, methane, nitrogen, carbon monoxide, oxygen, fluorine, argon, and carbon dioxide. The pressure range is generally from 0.1 to 400 atmospheres (to 100 atm for helium and to 1000 atm for hydrogen). The temperature ranges are from the triple point to 300 K for neon; to 500 K for carbon monoxide, oxygen, and fluorine; to 600 K for methane and nitrogen; to 1000 K for argon and carbon dioxide; to 2000 K for hydrogen; and from 6 to 500 K for helium. GASP accepts any two of pressure, temperature and density as input conditions along with pressure, and either entropy or enthalpy. The properties available in any combination as output include temperature, density, pressure, entropy, enthalpy, specific heats, sonic velocity, viscosity, thermal conductivity, and surface tension. The subprogram design is modular so that the user can choose only those subroutines necessary to the calculations.

  18. Broadening of the Spectral Atomic Lines Analysis in High Density Argon Corona Plasma by Using Voigt Profile

    Science.gov (United States)

    Nur, M.; Bonifaci, N.; Denat, A.; Atrazhev, V. M.

    2015-06-01

    Studies of spectrum emission from high density argon plasma corona has been done. The analysis of the boardening of spectral atomic lines of Ar-I profile has been curried out by using an empirical approximation based on a Voigt profile. Full-width at half-maximum (FWHM) of the spectral-lines of 763.5 nm has been determined from atmospheric pressure until liquid state. The study liquid argon was curried out in a variation of temperature from K to 151.2 K and hydrostatics pressure from 2.1 MPa to 6.4 MPa. These pressure gives the densities N∞ (i.e. density very far from ionization zone) a variation from 1.08 1022 to 2.11 1022 cm-3. FWHM of Voigt approximation (Wv) of the line 763,5 nm of 'Ar I for: the emission lamp very low pressure (Wv = 0,160 nm) and our corona discharge at a pressure of MPa (Wv = 0,67 nm) and at a pressure of 9,5 MPa (Wv = 1,16 nm). In gas, corona plasma has been generated from 0.1 MPa to 9.5 MPa. We found that the broadening spectral line increase by increasing densities both for. the spectral-lines of 763.5 nm and 696.5 nm. We concluded that broadening of spectrum cause of Van der Waals force.

  19. Broadening of the Interplanetary Helium Cone Structure Due to Elastic Collisions of LISM Helium Atoms with Solar Wind Ions

    Science.gov (United States)

    Fahr, H. J.; Nass, H. U.; Rucinski, D.

    1984-01-01

    Neutral interstellar particles penetrating into the heliosphere, besides being subject there to specific loss processes, suffer elastic collisions with KeV-solar wind ions. The momentum transfer to the neutrals connected with these collisions leads to a loss of angular momentum with respect to the Sun and to a fractional compensation of the effective solar gravity. The dynamical particle trajectories hence are changed into non-Keplerians leading to density and temperature distributions differing from those calculated in the past. This is found from a solution of the Boltzmann equation that linearizes the effect of this additional force. It is shown that the HeI-584A resonance glow of the heliospheric helium cone lead to substantially lower interstellar helium temperatures if re-interpreted on the basis of this revised theory. These temperatures now seem to be in accordance with the derived temperatures for interstellar hydrogen.

  20. An electron of helium atom under a high-intensity laser field

    Science.gov (United States)

    Falaye, Babatunde James; Sun, Guo-Hua; Adepoju, Adenike Grace; Liman, Muhammed S.; Oyewumi, K. J.; Dong, Shi-Hai

    2017-02-01

    We scrutinize the behavior of eigenvalues of an electron in a helium (He) atom as it interacts with electric field directed along the z-axis and is exposed to linearly polarized intense laser field radiation. To achieve this, we freeze one electron of the He atom at its ionic ground state and the motion of the second electron in the ion core is treated via a more general case of screened Coulomb potential model. Using the Kramers-Henneberger (KH) unitary transformation, which is the semiclassical counterpart of the Block-Nordsieck transformation in the quantized field formalism, the squared vector potential that appears in the equation of motion is eliminated and the resultant equation is expressed in the KH frame. Within this frame, the resulting potential and the corresponding wave function are expanded in Fourier series and using Ehlotzky’s approximation, we obtain a laser-dressed potential to simulate intense laser field. By fitting the more general case of screened Coulomb potential model into the laser-dressed potential, and then expanding it in Taylor series up to O≤ft({{r}4},α 09\\right) , we obtain the solution (eigenvalues and wave function) of an electron in a He atom under the influence of external electric field and high-intensity laser field, within the framework of perturbation theory formalism. We found that the variation in frequency of laser radiation has no effect on the eigenvalues of a He electron for a particular electric field intensity directed along z-axis. Also, for a very strong external electric field and an infinitesimal screening parameter, the system is strongly bound. This work has potential application in the areas of atomic and molecular processes in external fields including interactions with strong fields and short pulses.

  1. Calculations of Electron Structure of Endohedrally Confined Helium Atom with B-Spline Type Functions

    Institute of Scientific and Technical Information of China (English)

    QIAO HaoXue; SHI TingYun; LI BaiWen

    2002-01-01

    The B-spline basis set method is used to study the properties of helium confined endohedrally at thegeometrical centre of a fullerene. The boundary conditions of the wavefunctions can be simply satisfied with thismethod. From our results, the phenomenon of "mirror collapse" is found in the case of confining helium. The interestingbehaviors of confining helium are also discussed.

  2. Immobilization of single argon atoms in nano-cages of two-dimensional zeolite model systems

    Science.gov (United States)

    Zhong, Jian-Qiang; Wang, Mengen; Akter, Nusnin; Kestell, John D.; Boscoboinik, Alejandro M.; Kim, Taejin; Stacchiola, Dario J.; Lu, Deyu; Boscoboinik, J. Anibal

    2017-07-01

    The confinement of noble gases on nanostructured surfaces, in contrast to bulk materials, at non-cryogenic temperatures represents a formidable challenge. In this work, individual Ar atoms are trapped at 300 K in nano-cages consisting of (alumino)silicate hexagonal prisms forming a two-dimensional array on a planar surface. The trapping of Ar atoms is detected in situ using synchrotron-based ambient pressure X-ray photoelectron spectroscopy. The atoms remain in the cages upon heating to 400 K. The trapping and release of Ar is studied combining surface science methods and density functional theory calculations. While the frameworks stay intact with the inclusion of Ar atoms, the permeability of gasses (for example, CO) through them is significantly affected, making these structures also interesting candidates for tunable atomic and molecular sieves. These findings enable the study of individually confined noble gas atoms using surface science methods, opening up new opportunities for fundamental research.

  3. Immobilization of single argon atoms in nano-cages of two-dimensional zeolite model systems.

    Science.gov (United States)

    Zhong, Jian-Qiang; Wang, Mengen; Akter, Nusnin; Kestell, John D; Boscoboinik, Alejandro M; Kim, Taejin; Stacchiola, Dario J; Lu, Deyu; Boscoboinik, J Anibal

    2017-07-17

    The confinement of noble gases on nanostructured surfaces, in contrast to bulk materials, at non-cryogenic temperatures represents a formidable challenge. In this work, individual Ar atoms are trapped at 300 K in nano-cages consisting of (alumino)silicate hexagonal prisms forming a two-dimensional array on a planar surface. The trapping of Ar atoms is detected in situ using synchrotron-based ambient pressure X-ray photoelectron spectroscopy. The atoms remain in the cages upon heating to 400 K. The trapping and release of Ar is studied combining surface science methods and density functional theory calculations. While the frameworks stay intact with the inclusion of Ar atoms, the permeability of gasses (for example, CO) through them is significantly affected, making these structures also interesting candidates for tunable atomic and molecular sieves. These findings enable the study of individually confined noble gas atoms using surface science methods, opening up new opportunities for fundamental research.

  4. Zinc, lead and copper in human teeth measured by induced coupled argon plasma atomic emission spectroscopy (ICP-AES)

    Energy Technology Data Exchange (ETDEWEB)

    Chew, L.T.; Bradley, D.A. E-mail: D.A.Bradley@exeter.ac.uk; Mohd, Y.; Jamil, M

    2000-11-15

    Inductively Coupled Argon Plasma Atomic Emission Spectroscopy (ICP-AES) has been used to determine Pb, Zn and Cu levels in 47 exfoliated human teeth (all of which required extraction for orthodontic reasons). Lead concentrations for the group were 1.7 {mu}g (g tooth mass){sup -1} to 40.5 {mu}g (g tooth mass){sup -1}, with a median of 9.8 {mu}g (g tooth mass){sup -1}. A median lead level in excess of the group value was found for the teeth of six lorry drivers who were included in the study. A more significant enhancement was found for the seven subjects whose age was in excess of 60 years. The median values for Zn and Cu were 123.0 and 0.6 {mu}g (g tooth mass){sup -1} respectively. Present values for tooth-Zn are lower than published data for other ethnic groups.

  5. Variational Monte Carlo Studies of the Rate of Transmission of an Atomic Helium Beam through a Slab of Superfluid Helium by a Condensate Mediated Process

    Energy Technology Data Exchange (ETDEWEB)

    Setty, A.K.; Halley, J.W.; Campbell, C.E. [School of Physics and Astronomy, University of Minnesota, Minneapolis, Minnesota 55455 (United States)

    1997-11-01

    We report variational Monte Carlo calculations which give amplitudes and phases of the reflected and transmitted components of states representing scattering of helium atoms normally incident on a superfluid {sup 4}He slab. The wave function describes a previously postulated condensate mediated process [J.W. Halley {ital et al.,} Phys.Rev.Lett.{bold 71,} 2429 (1993)] and the results are consistent with uncertainty principle arguments suggesting that the transmission time for thin (but macroscopic) samples will be independent of slab thickness. {copyright} {ital 1997} {ital The American Physical Society}

  6. Shifts in the ESR spectra of alkali-metal atoms (Li, Na, K, Rb) on helium nanodroplets.

    Science.gov (United States)

    Hauser, Andreas W; Gruber, Thomas; Filatov, Michael; Ernst, Wolfgang E

    2013-03-18

    He-droplet-induced changes of the hyperfine structure constants of alkali-metal atoms are investigated by a combination of relativistically corrected ab initio methods with a simulation of the helium density distribution based on He density functional theory. Starting from an accurate description of the variation of the hyperfine structure constant in the M-He diatomic systems (M=Li, Na, K, Rb) as a function of the interatomic distance we simulate the shifts induced by droplets of up to 10,000 (4)He atoms. All theoretical predictions for the relative shifts in the isotropic hyperfine coupling constants of the alkali-metal atoms attached to helium droplets of different size are then tied to a single, experimentally derived parameter of Rb.

  7. Determination of {sup 233}U by inductively coupled argon plasma - atomic emission spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    Patwardhan, A.B.; Kulkarni, V.T.; Radhakrishnan, K.; Ramanujam, A.; Page, A.G. [Bhabha Atomic Research Centre, Bombay (India)

    1994-09-01

    The paper describes studies carried out for the determination of {sup 233}U at various stages during the recovery and purification of {sup 233}U from {sup 233}U-Al alloy scraps generated during the fabrication of {sup 233}U-Al alloy fuel. Employing a high resolution sequential spectrometer and Inductively Coupled argon Plasma (ICP) as the spectral excitation source, isotope shift for {sup 233}U with respect to {sup 238}U has been resolved and recorded. The shift for the 424.437 nm emission line of {sup 238}U is found to be of the order of 0.040 nm on the lower wavelength side for {sup 233}U and this isotopic effect has been utilised for the quantitative determination of {sup 233}U. The overall precision of the method is 5% RSD with the detection limit of 0.01 {mu}g/ml.

  8. Systematic effects in the measurement of the negatively charged pion mass using laser spectroscopy of pionic helium atoms

    CERN Document Server

    Obreshkov, Boyan

    2016-01-01

    The collision-induced shift and broadening of selected dipole transition lines of pionic helium in gaseous helium at low temperatures up to $T=12$ K and pressure up to a few bar are calculated within variable phase function approach. We predict blue shift of the resonance frequencies of the $(n,l)=(16,15) \\rightarrow (16,14) $ and $(16,15) \\rightarrow (17,14)$ unfavored transitions and red shift for the favored transition $(17,16) \\rightarrow (16,15)$. The result may be helpful in reducing the systematic error in proposed future experiments for determination of the negatively charged pion mass from laser spectroscopy of metastable pionic helium atoms.

  9. Antiprotonic helium

    CERN Multimedia

    Eades, John

    2005-01-01

    An exotic atom in w hich an electron and an antiproton orbit a helium nucleus could reveal if there are any differences between matter and antimatter. The author describes this unusual mirror on the antiworld (5 pages)

  10. Measurement of Absolute Atomic Collision Cross Section with Helium Using 87Rb Atoms Confined in Magneto-Optic and Magnetic Traps

    Institute of Scientific and Technical Information of China (English)

    WANG Ji-Cheng; ZHOU Ke-Ya; WANG Yue-Yuan; LIAO Qing-Hong; LIU Shu-Tian

    2011-01-01

    We present the measurements and calculations of the absolute total collision cross sections for a room-temperature gas of helium using 87 Rb atoms confined in either a magneto-optic or a magnetic quadrupole trap. The loss rates from the magneto-optic trap and the pure magnetic trap are compared and show significant differences. The collision cross sections as a function of trap depth for helium gas are obtained. These findings are significant for extracting the information about the different cross sections when the trap depth is changed.%@@ We present the measurements and calculations of the absolute total collision cross sections for a room-temperature gas of helium using 87Rb atoms confined in either a magneto-optic or a magnetic quadrupole trap.The loss rates from the magneto-optic trap and the pure magnetic trap are compared and show significant differences.The collision cross sections as a function of trap depth for helium gas are obtained.These findings are significant for extracting the information about the different cross sections when the trap depth is changed.

  11. Estimation of length scale of RS II-$p$ braneworld model through perturbations in Helium's atom ground state energy

    CERN Document Server

    Garrido, Nephtali

    2012-01-01

    We put to the test an effective three-dimensional electrostatic potential, obtained effectively by considering an electrostatic source inside a (5+$p$)-dimensional braneworld scenario with $p$ compact and one infinite spacial extra dimensions in the RS II-$p$ model, for $p=1$ and $p=2$. This potential is regular at the source and matches the standard Coulomb potential outside a neighborhood. We use variational and perturbative approximation methods to calculate corrections to the ground energy of the Helium atom modified by this potential, by making use of a 6 and 39-parameter trial wave function of Hylleraas type for the ground state. These corrections to the ground-state energy are compared with experimental data for Helium atom in order to set bounds for the extra dimensions length scale. We find that these bounds are less restrictive than the ones obtained by Morales et. al. through a calculation using the Lamb shift in Hydrogen.

  12. Role of Nuclear Coulomb Attraction in Nonsequential Double Ionization of Argon Atom

    Institute of Scientific and Technical Information of China (English)

    汤清彬; 张东玲; 李盈傧; 余本海

    2011-01-01

    The microscopic recollision dynamics in strong-field nonsequential double ionization of Ar atoms is in- vestigated using three-dimensional classical ensembles. By adjusting the nuclear Coulomb potential, we can excellently reproduce the experimental results both within the laser intensity regimes well above the reeollision threshold and well below the recollision threshold quantitatively. More importantly, our trajectory analysis clearly reveals the particular electronic dynamics in recollision process: the momentum of the recolliding electron encounters a sudden change both in magnitude and in direction when it approaches the nucleus closely, which show that the nuclear Coulomb attraction plays a key role in the recollision process of nonsequential double ionization of Ar atoms.

  13. Kinetic energy partition method applied to ground state helium-like atoms.

    Science.gov (United States)

    Chen, Yu-Hsin; Chao, Sheng D

    2017-03-28

    We have used the recently developed kinetic energy partition (KEP) method to solve the quantum eigenvalue problems for helium-like atoms and obtain precise ground state energies and wave-functions. The key to treating properly the electron-electron (repulsive) Coulomb potential energies for the KEP method to be applied is to introduce a "negative mass" term into the partitioned kinetic energy. A Hartree-like product wave-function from the subsystem wave-functions is used to form the initial trial function, and the variational search for the optimized adiabatic parameters leads to a precise ground state energy. This new approach sheds new light on the all-important problem of solving many-electron Schrödinger equations and hopefully opens a new way to predictive quantum chemistry. The results presented here give very promising evidence that an effective one-electron model can be used to represent a many-electron system, in the spirit of density functional theory.

  14. Penning ionization electron spectroscopy of hydrogen sulfide by metastable helium and neon atoms.

    Science.gov (United States)

    Falcinelli, Stefano; Candori, Pietro; Bettoni, Marta; Pirani, Fernando; Vecchiocattivi, Franco

    2014-08-21

    The dynamics of the Penning ionization of hydrogen sulfide molecules by collision with helium and metastable neon atoms, occurring in the thermal energy range, has been studied by analyzing the energy spectra of the emitted electrons obtained in our laboratory in a crossed beam experiment. These spectra are compared with the photoelectron spectra measured by using He(I) and Ne(I) photons under the same experimental conditions. In this way we obtained the negative energy shifts for the formation of H2S(+) ions in the first three accessible electronic states by He*(2(3,1)S1,0) and Ne*((3)P2,0) Penning ionization collisions: the 2b1 (X̃(2)B1) fundamental one, the first 5a1 (Ã(2)A1), and the second 2b2 (B̃(2)B2) excited states, respectively. The recorded energy shifts indicate that in the case of He* and Ne*-H2S the autoionization dynamics depends on the features of the collision complex and is mainly driven by an effective global attraction that comes from a balance among several non covalent intermolecular interaction components. This suggests that the Penning ionization should take place, in a specific range of intermolecular distances, as we have already observed in the case of Penning ionization of water molecules [Brunetti, B. G.; Candori, P.; Falcinelli, S.; Pirani, F.; Vecchiocattivi, F. J. Chem. Phys. 2013, 139, 164305-1-164305-8].

  15. Luminescence of atomic magnesium in inert low temperature solids. I. Argon and krypton

    Science.gov (United States)

    McCaffrey, John G.; Ozin, Geoffrey A.

    1994-12-01

    Absorption and luminescence spectra have been recorded in the 200-700 nm range for atomic magnesium isolated in solid Ar and Kr at 12 K. Strong absorptions occurring in the near UV at 285 nm, showing a threefold splitting, are identified as the solid phase equivalent of the gas phase 3p 1P1←3s 1S0 Mg atom transition. Evidence of multiple site trapping of Mg atoms in Ar and Kr matrices formed at 12 K has been obtained from annealing studies in absorption, but especially in luminescence spectroscopy. The single emission band of Mg/Ar, centered at 297.6 nm, exhibits a radiative lifetime of 1.12 ns and is thereby assigned as singlet 3p 1P1→3s 1S0 Mg atom fluorescence. The luminescence exhibited by the Mg/Kr system is more complex than the Mg/Ar system in that a weak visible band at 472 nm occurs as well as several bands in the UV having nanosecond lifetimes. The richness of the Mg/Kr UV spectra has been examined with annealing and time-resolved measurements and identified as arising from multiple trapping site effects, with at least three spectrally distinct sites identified. Efficient resonant radiative energy transfer is demonstrated to be occurring between two of these sites and an average separation between the sensitizor and activator sites is calculated to be 60 nm at a Mg:Ar dilution ratio of 3:104. Annealing of Mg/Kr samples to 45 K was found to remove all but one site which exhibits emission at 297.6 nm and a very weak band at 472.6 nm. The former, having a radiative lifetime of 1.25 ns, is assigned as 3p 1P1→3s 1S0 Mg atom fluorescence; the latter with a radiative lifetime of 8.9 ms, is assigned as 3p 3P1→3s 1S0 Mg atom phosphorescence.

  16. Magnetic resonance studies of atomic hydrogen at zero field and low temperature. Recombination and binding on liquid helium

    Energy Technology Data Exchange (ETDEWEB)

    Jochemsen, R.; Morrow, M.; Berlinsky, A.J.; Hardy, W.N. (British Columbia Univ., Vancouver (Canada). Dept. of Physics)

    1982-07-01

    Magnetic resonance studies at zero field are reported for atomic hydrogen gas confined in a closed glass bulb with helium-coated walls for T<1 K in a dilution refrigerator. Low-energy r.f. discharge pulses have been used to produce H atoms at temperatures as low as T=0.06 K. The atom density nsub(H) (10/sup 9/..H/sub 2/+wall. From the temperature dependence of the rate constant K we have determined the binding energy of H on liquid /sup 4/He and /sup 3/He, and also the cross section for recombination on the surface.

  17. One- and two-photon spectroscopy of highly excited states of alkali-metal atoms on helium nanodroplets.

    Science.gov (United States)

    Pifrader, Alexandra; Allard, Olivier; Auböck, Gerald; Callegari, Carlo; Ernst, Wolfgang E; Huber, Robert; Ancilotto, Francesco

    2010-10-28

    Alkali-metal atoms captured on the surface of superfluid helium droplets are excited to high energies (≈3 eV) by means of pulsed lasers, and their laser-induced-fluorescence spectra are recorded. We report on the one-photon excitation of the (n+1)p←ns transition of K, Rb, and Cs (n=4, 5, and 6, respectively) and on the two-photon one-color excitation of the 5d←5s transition of Rb. Gated-photon-counting measurements are consistent with the relaxation rates of the bare atoms, hence consistent with the reasonable expectation that atoms quickly desorb from the droplet and droplet-induced relaxation need not be invoked.

  18. Room-temperature atomic layer deposition of ZrO{sub 2} using tetrakis(ethylmethylamino)zirconium and plasma-excited humidified argon

    Energy Technology Data Exchange (ETDEWEB)

    Kanomata, K. [Graduate School of Science and Engineering, Yamagata University, 4-3-16 Jonan, Yonezawa 992-8510 (Japan); Japan Society for the Promotion of Science, 5-3-1 Kojimachi, Chiyoda-ku, Tokyo 102-0083 (Japan); Tokoro, K.; Imai, T.; Pansila, P.; Miura, M.; Ahmmad, B.; Kubota, S.; Hirahara, K. [Graduate School of Science and Engineering, Yamagata University, 4-3-16 Jonan, Yonezawa 992-8510 (Japan); Hirose, F., E-mail: fhirose@yz.yamagata-u.ac.jp [Graduate School of Science and Engineering, Yamagata University, 4-3-16 Jonan, Yonezawa 992-8510 (Japan)

    2016-11-30

    Highlights: • RT-ALD of ZrO{sub 2} is developed using TEMAZ and plasma-excited humidified argon. • The plasma-excited humidified argon is effective in oxidizing the TEMAZ saturated ZrO{sub 2}. • We discuss the reaction mechanism of the RT-ZrO{sub 2} ALD. - Abstract: Room-temperature atomic layer deposition (ALD) of ZrO{sub 2} is developed with tetrakis(ethylmethylamino)zirconium (TEMAZ) and a plasma-excited humidified argon. A growth per cycle of 0.17 nm/cycle at room temperature is confirmed, and the TEMAZ adsorption and its oxidization on ZrO{sub 2} are characterized by IR absorption spectroscopy with a multiple internal reflection mode. TEMAZ is saturated on a ZrO{sub 2} surface with exposures exceeding ∼2.0 × 10{sup 5} Langmuir (1 Langmuir = 1.0 × 10{sup −6} Torr s) at room temperature, and the plasma-excited humidified argon is effective in oxidizing the TEMAZ-adsorbed ZrO{sub 2} surface. The IR absorption spectroscopy suggests that Zr-OH works as an adsorption site for TEMAZ. The reaction mechanism of room-temperature ZrO{sub 2} ALD is discussed in this paper.

  19. LIF Measurements on an Atomic Helium Beam in the Edge of a Fusion Plasma—possible derivation of the electron density

    Science.gov (United States)

    Krychowiak, M.; Mertens, Ph.; Schweer, B.; Brezinsek, S.; König, R.; Schmitz, O.; Brix, M.; Klinger, T.; Samm, U.

    2008-03-01

    Local values of the electron density and temperature in the edge of a fusion plasma can be derived with high space and time resolution by the use of line radiation of atomic helium beams. The accuracy of this method is mainly limited by the uncertainties in the collisional-radiative model which is needed in order to obtain both plasma parameters from the measured relative intensities of atomic helium lines. Combination of a helium beam with a pulsed high-power laser provides a possibility of ne measurement which does not require a detailed knowledge of the collisional-radiative model. The method relies on resonant laser pumping of some levels and analyzing their fluorescence after the end of the laser pulse. Such measurements were already performed in low temperature plasmas with some content of atomic helium [1,2,3]. In this paper, we discuss the applicability of this method in the fusion edge plasma in the density range of ˜1012-1013 cm-3 when exciting helium atoms with a laser at the wavelength of λ = 388.9 nm tuned to the triplet transition 23S⃗33P ° and observing the fluorescence light at the laser wavelength and at λ = 587.6 nm(33D⃗23P °). A first test measurement at the TEXTOR tokamak in Jülich performed by use of an excimer-pumped dye laser in connection with a thermal helium beam is shown and discussed.

  20. Calculation of Energies of the Ground and Low Excited States of a Confined Helium Atom in a Spherical Parabolic Well

    Institute of Scientific and Technical Information of China (English)

    XIE Wen-Fang

    2006-01-01

    @@ Making use of the adiabatic hyperspherical approach, we report a calculation for the energy spectrum of the ground and low-excited states of the confined helium atom in a spherical parabolic well. We find that the energies of a spherical parabolic well are in good agreement with those of an impenetrable spherical box for the larger confined potential radius. However, the energy values of a spherical parabolic well are much lower than those of an impenetrable spherical box for small values of re. We also find that the confinement may cause accidental degeneracies between levels with different low-excited states and the inversion of the energy values.

  1. Influences of the propyl group on the van der Waals structures of 4-propylaniline complexes with one and two argon atoms studied by electronic and cationic spectroscopy

    Science.gov (United States)

    Yang, Zhijun; Gu, Quanli; Trindle, Carl O.; Knee, J. L.

    2015-07-01

    4-propylaniline complexes with one and two argon atoms formed in the molecular beam were studied in the first excited electronic state, S1, using resonance enhanced two-photon ionization spectroscopy and in the cation ground state, D0, using mass analyzed threshold ionization spectroscopy. The combination of electronic and cationic spectra of the clusters allows two conformations to be identified in both aniline-Ar1 and aniline-Ar2, which are assigned to either the gauche configuration or anti-configuration of 4-propylaniline. The gauche isomer exhibits complex bands shifted 29 cm-1 and 89 cm-1 from the S1 origin bands and 83 cm-1 and 148 cm-1 from the ionization potential assigned to the Ar1 and Ar2 complexes, respectively. For the anti-rotamer, the corresponding shifts actually become nearly additive, 53 cm-1 and 109 cm-1 for the S1 origin bands, and 61 cm-1 and 125 cm-1 for the ionization potentials. Ab initio calculations provide insights into the influences of the propyl and amino groups on the positions of the argon atoms within the clusters. In addition, the binding energy of one argon with the gauche isomer of 4-propylaniline has been measured to be 550 ± 5 cm-1 in the D0 state, 496 ± 5 cm-1 in the S1 state, and 467 ± 5 cm-1 in the neutral ground state, S0.

  2. Room-temperature atomic layer deposition of ZrO2 using tetrakis(ethylmethylamino)zirconium and plasma-excited humidified argon

    Science.gov (United States)

    Kanomata, K.; Tokoro, K.; Imai, T.; Pansila, P.; Miura, M.; Ahmmad, B.; Kubota, S.; Hirahara, K.; Hirose, F.

    2016-11-01

    Room-temperature atomic layer deposition (ALD) of ZrO2 is developed with tetrakis(ethylmethylamino)zirconium (TEMAZ) and a plasma-excited humidified argon. A growth per cycle of 0.17 nm/cycle at room temperature is confirmed, and the TEMAZ adsorption and its oxidization on ZrO2 are characterized by IR absorption spectroscopy with a multiple internal reflection mode. TEMAZ is saturated on a ZrO2 surface with exposures exceeding ∼2.0 × 105 Langmuir (1 Langmuir = 1.0 × 10-6 Torr s) at room temperature, and the plasma-excited humidified argon is effective in oxidizing the TEMAZ-adsorbed ZrO2 surface. The IR absorption spectroscopy suggests that Zr-OH works as an adsorption site for TEMAZ. The reaction mechanism of room-temperature ZrO2 ALD is discussed in this paper.

  3. Influence of ion-to-atom ratio on the microstructure of evaporated molybdenum thin films grown using low energy argon ions

    Energy Technology Data Exchange (ETDEWEB)

    Yadav, Praveen Kumar, E-mail: praveenyadav@rrcat.gov.in; Nayak, Maheswar; Rai, Sanjay Kumar; Lodha, Gyanendra Singh [X-ray Optics Section, Indus Synchrotrons Utilization Division, Raja Ramanna Centre for Advanced Technology, Indore 452013 (India); Sant, Tushar; Sharma, Surinder Mohan [High Pressure and Synchrotron Radiation Physics Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Mukherjee, Chandrachur [Mechanical and Optical Support Section, Raja Ramanna Centre for Advanced Technology, Indore 452013 (India)

    2014-03-15

    The authors report the effect of argon ion to molybdenum atom ratio (r) on the microstructure of low energy (70 eV) argon ion assisted electron beam evaporated Mo thin films. Surface roughness, morphology, and crystallinity of Mo films are found to strongly depend on “r.” Increase of “r” from 0 to 100 induces gradual loss in crystallinity, reduction in surface roughness and systematic increase in density of the film. For “r” ∼ 100, average atomic density of the film approaches the bulk value (97%) with lowest surface roughness. Further, increasing “r” up to 170 reduces the atomic density, increases roughness, and increase in crystallinity induced by low energy Ar ion beam. The observed surface roughness and grain size determined by x-ray reflectivity and glancing incidence x-ray diffraction correlate well with atomic force microscopy measurements. This study demonstrates that for r = 100 one gets lowest roughness Mo film with highest density and nearly amorphous microstructure. The growth model is discussed by structural zone model.

  4. Triple differential cross section for the near threshold single ionization of helium atoms for equal energy sharing

    Energy Technology Data Exchange (ETDEWEB)

    Purohit, G., E-mail: ghanshyam.purohit@spsu.ac.in [Department of Physics, School of Engineering, Sir Padampat Singhania University, Bhatewar, Udaipur 313 601 (India); Singh, P. [Department of Physics, School of Engineering, Sir Padampat Singhania University, Bhatewar, Udaipur 313 601 (India); Dorn, A.; Ren, X. [Max Planck Institute for Nuclear Physics, 69117 Heidelberg (Germany); Patidar, V. [Department of Physics, School of Engineering, Sir Padampat Singhania University, Bhatewar, Udaipur 313 601 (India)

    2016-05-15

    Highlights: • Present paper describes electron impact single ionization of helium atoms near threshold. • This energy range provided challenges to theoretical models due to presence of several physical effects at low energies such as second order processes, PCI, polarization, etc. • Inclusion of second Born term and target polarization is helpful to analyze the measurements. • Present paper also describes usefulness of post collisional interaction in the collision dynamics at low energies. - Abstract: Low energy electron impact single ionization triple differential cross section (TDCS) results are reported for the helium atoms in the threshold regime at 1 eV, 3 eV and 5 eV excess energy. TDCSs are calculated in the doubly symmetric kinematics for the coplanar to perpendicular emission of electrons. Present attempt to calculate TDCS in the second Born approximation and treating target polarization and post collision interaction is helpful to analyze the available measurements. The second order processes, target polarization and post collision interaction (PCI) have been found to be significant in describing the trends of TDCS and helpful to produce reasonably good agreement with measurements.

  5. Wigner’s phase-space function and atomic structure: II. Ground states for closed-shell atoms

    DEFF Research Database (Denmark)

    Springborg, Michael; Dahl, Jens Peder

    1987-01-01

    display and analyze the function for the closed-shell atoms helium, beryllium, neon, argon, and zinc in the Hartree-Fock approximation. The quantum-mechanical exact results are compared with those obtained with the approximate Thomas-Fermi description of electron densities in phase space....

  6. On the difference between breakdown and quench voltages of argon plasma and its relation to $4p-4s$ atomic state transitions

    CERN Document Server

    Forati, Ebrahim; Sievenpiper, Dan

    2014-01-01

    Using a relaxation oscillator circuit, breakdown ($V_{\\mathrm{BD}}$) and quench ($V_{\\mathrm{Q}}$) voltages of a DC discharge microplasma between two needle probes are measured. High resolution modified Paschen curves are obtained for argon microplasmas including a quench voltage curve representing the voltage at which the plasma turns off. It is shown that, for a point to point microgap (e.g. the microgap between two needle probes) which describes many realistic microdevices, neither Paschen's law applies nor field emission is noticeable. Although normally $V_{\\mathrm{BD}}>V_{\\mathrm{Q}}$, it is observed that depending on environmental parameters of argon, such as pressure and the driving circuitry, plasma can exist in a different state with equal $V_{\\mathrm{BD}}$ and $V_{\\mathrm{Q}}$. Using emission line spectroscopy, it is shown that $V_{\\mathrm{BD}}$ and $V_{\\mathrm{Q}}$ are equal if the atomic excitation by the electric field dipole moment dominantly leads to one of the argon's metastable states ($4P_{5...

  7. On the difference between breakdown and quench voltages of argon plasma and its relation to 4p–4s atomic state transitions

    Energy Technology Data Exchange (ETDEWEB)

    Forati, Ebrahim, E-mail: forati@ieee.org; Piltan, Shiva; Sievenpiper, Dan, E-mail: dsievenpiper@ucsd.edu [University of California San Diego, La Jolla, California 92093 (United States)

    2015-02-02

    Using a relaxation oscillator circuit, breakdown (V{sub BD}) and quench (V{sub Q}) voltages of a DC discharge microplasma between two needle probes are measured. High resolution modified Paschen curves are obtained for argon microplasmas including a quench voltage curve representing the voltage at which the plasma turns off. It is shown that for a point to point microgap (e.g., the microgap between two needle probes) which describes many realistic microdevices, neither Paschen's law applies nor field emission is noticeable. Although normally V{sub BD} > V{sub Q,} it is observed that depending on environmental parameters of argon, such as pressure and the driving circuitry, plasma can exist in a different state with equal V{sub BD} and V{sub Q.} Using emission line spectroscopy, it is shown that V{sub BD} and V{sub Q} are equal if the atomic excitation by the electric field dipole moment dominantly leads to one of the argon's metastable states (4P{sub 5} in our study)

  8. Atomic oxygen in a cold argon plasma jet: TALIF spectroscopy in ambient air with modelling and measurements of ambient species diffusion

    Science.gov (United States)

    Reuter, S.; Winter, J.; Schmidt-Bleker, A.; Schroeder, D.; Lange, H.; Knake, N.; Schulz-von der Gathen, V.; Weltmann, K.-D.

    2012-04-01

    By investigating the atomic oxygen density in its effluent, two-photon absorption laser-induced fluorescence (TALIF) spectroscopy measurements are for the first time performed in a cold argon/oxygen atmospheric pressure plasma jet. The measurements are carried out in ambient air and quenching by inflowing air species is considered. We propose a novel absorption technique in the VUV spectral range, where emission originating from within the discharge is used as light source to determine the inflow of atmospheric oxygen into the effluent. Furthermore, we propose a modelling solution for the on-axis density of inflowing ambient air based on the stationary convection-diffusion equation.

  9. Formation of Exotic Networks of Water Clusters in Helium Droplets Facilitated by the Presence of Neon Atoms

    Energy Technology Data Exchange (ETDEWEB)

    Douberly, Gary E.; Miller, Roger E.; Xantheas, Sotiris S.

    2017-03-08

    Water clusters are formed in helium droplets via the sequential capture of monomers. One or two neon atoms are added to each droplet prior to the addition of water. The infrared spectrum of the droplet ensemble reveals several signatures of polar, water tetramer clusters having dipole moments between 2D and 3D. Comparison with ab initio computations supports the assignment of the cluster networks to noncyclic “3+1” clusters, which are ~5.3 kcal/mol less stable than the global minimum nonpolar cyclic tetramer. The (H2O)3Ne + H2O ring insertion barrier is sufficiently large, such that evaporative helium cooling is capable of kinetically quenching the nonequilibrium tetramer system prior to its rearrangement to the lower energy cyclic species. To this end, the reported process results in the formation of exotic water cluster networks that are either higher in energy than the most stable gas-phase analogs or not even stable in the gas phase.

  10. Formation of Exotic Networks of Water Clusters in Helium Droplets Facilitated by the Presence of Neon Atoms.

    Science.gov (United States)

    Douberly, Gary E; Miller, Roger E; Xantheas, Sotiris S

    2017-03-22

    Water clusters are formed in helium droplets via the sequential capture of monomers. One or two neon atoms are added to each droplet prior to the addition of water. The infrared spectrum of the droplet ensemble reveals several signatures of polar, water tetramer clusters having dipole moments between 2D and 3D. Comparison with ab initio computations supports the assignment of the cluster networks to noncyclic "3 + 1" clusters, which are ∼5.3 kcal/mol less stable than the global minimum nonpolar cyclic tetramer. The (H2O)3Ne + H2O ring insertion barrier is sufficiently large, such that evaporative helium cooling is capable of kinetically quenching the nonequilibrium tetramer system prior to its rearrangement to the lower energy cyclic species. To this end, the reported process results in the formation of exotic water cluster networks that are either higher in energy than the most stable gas-phase analogs or not even stable in the gas phase.

  11. Influences of the propyl group on the van der Waals structures of 4-propylaniline complexes with one and two argon atoms studied by electronic and cationic spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Yang, Zhijun [School of Basic Medical Sciences, Xinxiang Medical University, Xinxiang, Henan 453003 (China); Gu, Quanli [School of Basic Medical Sciences, Xinxiang Medical University, Xinxiang, Henan 453003 (China); Department of Chemistry, University of Oklahoma, Norman, Oklahoma 73019 (United States); Trindle, Carl O., E-mail: cot@virginia.edu [Chemistry Department, University of Virginia, Charlottesville, Virginia 22904 (United States); Knee, J. L., E-mail: jknee@wesleyan.edu [Chemistry Department, Wesleyan University, Middletown, Connecticut 06459 (United States)

    2015-07-21

    4-propylaniline complexes with one and two argon atoms formed in the molecular beam were studied in the first excited electronic state, S{sub 1}, using resonance enhanced two-photon ionization spectroscopy and in the cation ground state, D{sub 0}, using mass analyzed threshold ionization spectroscopy. The combination of electronic and cationic spectra of the clusters allows two conformations to be identified in both aniline-Ar{sub 1} and aniline-Ar{sub 2}, which are assigned to either the gauche configuration or anti-configuration of 4-propylaniline. The gauche isomer exhibits complex bands shifted 29 cm{sup −1} and 89 cm{sup −1} from the S{sub 1} origin bands and 83 cm{sup −1} and 148 cm{sup −1} from the ionization potential assigned to the Ar{sub 1} and Ar{sub 2} complexes, respectively. For the anti-rotamer, the corresponding shifts actually become nearly additive, 53 cm{sup −1} and 109 cm{sup −1} for the S{sub 1} origin bands, and 61 cm{sup −1} and 125 cm{sup −1} for the ionization potentials. Ab initio calculations provide insights into the influences of the propyl and amino groups on the positions of the argon atoms within the clusters. In addition, the binding energy of one argon with the gauche isomer of 4-propylaniline has been measured to be 550 ± 5 cm{sup −1} in the D{sub 0} state, 496 ± 5 cm{sup −1} in the S{sub 1} state, and 467 ± 5 cm{sup −1} in the neutral ground state, S{sub 0}.

  12. Helium Energetic Neutral Atoms - a New Perspective for Heliospheric and Extraheliospheric Observations with IMAP

    Science.gov (United States)

    Swaczyna, P.; Grzedzielski, S.; Bzowski, M.

    2015-12-01

    Helium as the second most abundant species in the solar wind as well as in the interstellar medium should be prominent in the observations made be ENA detectors. Since IBEX-Hi detector was not equipped with a mass spectrometer, He ENA contribute only negligibly to the overall signal observed with the detector and are indistinguishable from the hydrogen ENAs. The situation will likely change with the ENA detector on IMAP. In our work we assess the expected heliospheric and potential extraheliospheric emission of He ENAs and show potential ability of He ENAs to resolve the structure of the LISM in the proximity of the heliosphere. We assess the heliospheric emission using a simple model of the heliosphere that takes the Voyager observations into account. We assume helium ion spectra at the termination shock and propagate them through the inner heliosheath. The computed distributions are then used to integrate the He ENA fluxes. To assess the IBEX Ribbon emission we adapt the analytical model of the Secondary ENA emission by Moebius et al. 2013 for helium. We obtain that both the inner heliosheath and the Ribbon emissions are much weaker than the observed H ENA by IBEX, except from the heliotail. One of the possible explanations for the IBEX Ribbon proposed by Grzedzielski et al. 2010 suggests that the signal originates in the boundary region between the LIC and the cavity of the Local Bubble. The main disadvantage of the model is the necessity of a short distance to this interface and low plasma density in the LIC, so that ionization processes do not extinct the signal. However, the mean free path for He ENAs ionization could be longer by an order of magnitude and reaches about 8000 AU. This should allow us to observe ENAs originating from suprathermal ions created in processes likely operating at the LIC boundaries, the distance to which could be ~0.1 pc. This makes He ENA observations a unique tool to observe such regions, currently inaccessible to optical

  13. Dynamic polarizabilities of rare-earth-metal atoms and dispersion coefficients for their interaction with helium atoms

    NARCIS (Netherlands)

    Chu, X.; Dalgarno, A.; Groenenboom, G.C.

    2007-01-01

    The dynamic scalar and tensor polarizabilities of the rare-earth-metal atoms are calculated with time-dependent density functional theory. The frequency-dependent polarizabilities at imaginary frequencies are used to determine the isotropic and orientation-dependent van der Waals coefficients for th

  14. Migration and nucleation of helium atoms at (110) twist grain boundaries in tungsten

    Science.gov (United States)

    Feng, Ya-Xin; Shang, Jia-Xiang; Lu, Guang-Hong

    2017-04-01

    The migration and nucleation of He atoms at three typical (110) twist grain boundaries (TGBs): the low-angle grain boundary (LAGB), the ordinary high-angle grain boundary (HAGB) and the Σ 3 TGB in W are investigated using molecular dynamics simulations. The presence of TGBs can absorb He atoms from bulk and impede the growth of He bubbles. Moreover, different grain boundary (GB) structures behave differently when interacting with He atoms. The LAGB can control the He distribution on the GB plane through its screw dislocation network, suggesting a promising approach for design of radiation tolerant materials. The ordinary HAGB presents a strong trap effect due to its disordered GB structure, which may induce a large He retention at the GB and embrittlement. The Σ 3 TGB can provide a diffusion path for He atoms, although the diffusion rate is not as fast as it in bulk.

  15. Long-range interactions between excited helium and alkali-metal atoms

    KAUST Repository

    Zhang, J.-Y.

    2012-12-03

    The dispersion coefficients for the long-range interaction of the first four excited states of He, i.e., He(2 1,3S) and He(2 1,3P), with the low-lying states of the alkali-metal atoms Li, Na, K, and Rb are calculated by summing over the reduced matrix elements of the multipole transition operators. For the interaction between He and Li the uncertainty of the calculations is 0.1–0.5%. For interactions with other alkali-metal atoms the uncertainty is 1–3% in the coefficient C5, 1–5% in the coefficient C6, and 1–10% in the coefficients C8 and C10. The dispersion coefficients Cn for the interaction of He(2 1,3S) and He(2 1,3P) with the ground-state alkali-metal atoms and for the interaction of He(2 1,3S) with the alkali-metal atoms in their first 2P states are presented in this Brief Report. The coefficients for other pairs of atomic states are listed in the Supplemental Material.

  16. Energy Levels in Helium and Neon Atoms by an Electron-Impact Method.

    Science.gov (United States)

    Taylor, N.; And Others

    1981-01-01

    Electronic energy levels in noble gas atoms may be determined with a simple teaching apparatus incorporating a resonance potentials tube in which the electron beam intensity is held constant. The resulting spectra are little inferior to those obtained by more elaborate electron-impact methods and complement optical emission spectra. (Author/SK)

  17. Deviation from Boltzmann distribution in excited energy levels of singly-ionized iron in an argon glow discharge plasma for atomic emission spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    Zhang Lei; Kashiwakura, Shunsuke; Wagatsuma, Kazuaki, E-mail: wagatuma@imr.tohoku.ac.jp

    2012-01-15

    A Boltzmann plot for many iron ionic lines having excitation energies of 4.7-9.1 eV was investigated in an argon glow discharge plasma when the discharge parameters, such as the voltage/current and the gas pressure, were varied. A Grimm-style radiation source was employed in a DC voltage range of 400-800 V at argon pressures of 400-930 Pa. The plot did not follow a linear relationship over a wide range of the excitation energy, but it yielded a normal Boltzmann distribution in the range of 4.7-5.8 eV and a large overpopulation in higher-lying excitation levels of iron ion. A probable reason for this phenomenon is that excitations for higher excited energy levels of iron ion would be predominantly caused by non-thermal collisions with argon species, the internal energy of which is received by iron atoms for the ionization. Particular intense ionic lines, which gave a maximum peak of the Boltzmann plot, were observed at an excitation energy of ca. 7.7 eV. They were the Fe II 257.297-nm and the Fe II 258.111-nm lines, derived from the 3d{sup 5}4s4p {sup 6}P excited levels. The 3d{sup 5}4s4p {sup 6}P excited levels can be highly populated through a resonance charge transfer from the ground state of argon ion, because of good matching in the excitation energy as well as the conservation of the total spin before and after the collision. An enhancement factor of the emission intensity for various Fe II lines could be obtained from a deviation from the normal Boltzmann plot, which comprised the emission lines of 4.7-5.8 eV. It would roughly correspond to a contribution of the charge transfer excitation to the excited levels of iron ion, suggesting that the charge-transfer collision could elevate the number density of the corresponding excited levels by a factor of ca.10{sup 4}. The Boltzmann plots give important information on the reason why a variety of iron ionic lines can be emitted from glow discharge plasmas.

  18. Non-dispersive atomic-fluorescence spectrometry of trace amounts of bismuth by introduction of its gaseous hydride into a premixed argon (entrained air)-hydrogen flame.

    Science.gov (United States)

    Kobayashi, S; Nakahara, T; Musha, S

    1979-10-01

    A method has been developed for the determination of bismuth by generation of its gaseous hydride and introduction of the hydride into a premixed argon (entrained air)-hydrogen flame, the atomic-fluorescence lines from which are all detected by use of a non-dispersive system. The detection limit is 5 pg/ml, or 0.1 ng of bismuth, but the reagent blank found in a 20-ml sample volume was approximately 2 ng of bismuth. Analytical working curves obtained by measuring peak-heights and integrated peak-areas of the signals are linear over a range of about four orders of magnitude from the detection limit. Perchloric, phosphoric and sulphuric acids up to 2.0M concentration give no interference, but nitric acid gives slight depression of the signal. The presence of silver, gold, nickel, palladium, platinum, selenium and tellurium in 1000-fold ratio to bismuth causes pronounced depression of the signal, whereas mercury and tin slightly enhance the atomic-fluorescence signal. The method has been applied to the determination of bismuth in aluminium-base alloys and sulphide ores with use of the standard additions method. The results are in good agreement with those obtained by flame atomic-absorption spectrometry and optical emission spectrometry with an inductively coupled plasma.

  19. Analysis of the excited argon atoms in the GEC RF reference cell by means of one-dimensional PIC simulations

    Energy Technology Data Exchange (ETDEWEB)

    Lauro-Taroni, L [The Open University, Oxford Research Unit, Oxford, OX1 5HR (United Kingdom); Turner, M M [Plasma Research Laboratory, School of Physical Sciences and National Centre for Plasma Science and Technology, Dublin City University, Dublin (Ireland); Braithwaite, N StJ [Open University, Oxford Research Unit, Oxford, OX1 5HR (United Kingdom)

    2004-08-21

    We examine the question of whether the excited states in argon contribute significantly to ionization in a capacitively coupled plasma through metastable pooling and step-ionization processes. We look at this issue by means of a one-dimensional particle-in-cell (PIC) code, with collisions treated by a Monte Carlo collision package. In the range explored, 50-1000 mTorr, the main source of ionization, in the absence of secondary emission, is direct ionization from the ground state with a contribution from excited states that is negligible at lower pressures, but increases in importance at higher pressures. When secondary electrons are included, their interaction with ground state neutrals dominates the ionization. At higher pressures the metastable profiles can reveal useful information on the non-uniform mean electron energy across the discharge, even though these states do not necessarily play a significant role in ionization.

  20. Partial Wave Cross Sections for Collisions between Helium Atoms and Hydrogen Halide Molecules

    Institute of Scientific and Technical Information of China (English)

    YU Chun-Ri; CHENG Xin-Lu; YANG Xiang-Dong

    2007-01-01

    The close-coupling method is utilized to calculate partial cross sections for elastic and inelastic scattering of He atoms with HX (X=F, Cl, Br) molecule based on the CCSD (T) potential energy surfaces obtained in the previous research. The calculation is performed at the incident energy of 200 me V. The rationality of our results has been confirmed by comparison with the available theoretical results. The tendency of the elastic and inelastic rotational excitation partial wave cross sections varying with the reduced mass of the three systems is obtained.

  1. The direct ionization processes in the collisions of partially stripped carbon and oxygen ions with helium atoms at low-to-intermediate energies

    Institute of Scientific and Technical Information of China (English)

    Zhou Chun-Lin; Shao Jian-Xiong; Chen Xi-Meng; Sun Guang-Zhi; Zou Xian-Rong

    2008-01-01

    The values of direct double- to-single ionization ratio R of helium atoms induced by Cq+,Oq+ (q=1-4) ions at incident energies from 0.2 to 8.5MeV are measured.Based on the existing model (Shao J X,Chen X M and Ding B W 2007 Phys.Rev.A 75 012701) the effective charge of the projectile is introduced to theoretically estimate the value of R for the partially stripped ions impacting on helium atoms.The results calculated from our "effective charge" model are in good agreement with the experimental data,and the dependence of the effective charge on the ionization energy of the projectile is also discussed qualitatively.

  2. Atom probe field ion microscope study of the range and diffusivity of helium in tungsten

    Energy Technology Data Exchange (ETDEWEB)

    Wagner, A.

    1978-08-01

    A time-of-flight (TOF) atom-probe field-ion microscope (FIM) specifically designed for the study of defects in metals is described. With this automated system 600 TOF min/sup -1/ can be recorded and analyzed. Performance tests of the instrument demonstrated that (1) the seven isotopes of molybdenum and the five isotopes of tungsten can be clearly resolved; and (2) the concentration and spatial distribution of all constitutents present at levels greater than 0.05 at. % in a W--25 at. % Re, Mo--1.0 at. % Ti, Mo--1.0 at. % Ti--0.08 at. % Zr (TZM), a low swelling stainless steel (LS1A) and a metallic glass (Metglas 2826) can be measured. The effect of the rate of field evaporation on the quantitative atom probe analysis of a Mo--1.0 at. % Ti alloy and a Mo--1.0 at. % Ti--0.08 at. % Zr alloy was investigated. As the field evaporation rate increased the measured Ti concentration was found to also increase. A simple qualitative model was proposed to explain the observation. The spatial distribution of titanium in a fast neutron irradiated Mo--1.0 at. % Ti alloy has been investigated. No evidence of Ti segregation to the voids was detected nor has any evidence of significant resolution of Ti from the TiC precipitates been detected. A small amount of segregation of carbon to a void was detected.

  3. Efficacy of argon-helium cryosurgery for gliomas in 9L/Fischer344 rats%氩氦冷冻治疗9L/Fischer344大鼠脑胶质瘤疗效观察

    Institute of Scientific and Technical Information of China (English)

    刘剑; 马国亮; 夏爱祥; 张世忠; 黄传平; 林武鹏; 王德才

    2013-01-01

    Objective To research the efficacy of argon-helium cryotherapy for glioma and the prognosis in 9L/Fischer344 rats.Methods Fischer344 rat glioma models were successfully established and divided into blank control group,surgery group and cryotherapy group,10 rats each.The size of the tumor was measured and calculated by vemier caliper.The behavior and survival of rats was observed before and atter cryotherapy.Results The survival time in blank control group,surgery group and cryotherapy group was 78.5±1.1,171.0±10.8 and 252.8±5.0 days respectively,and the difference was statistically significant (P =0.002).The tumor volume showed a trend to decrease in cryotherapy group.Conclusions Cryosurgery is an effective treatment for glioma,presumably due to the tumor cell rupture-caused antigen exposure stimulating the body to produce anti-tumor antibodies.%目的 研究氩氦冷冻治疗9L/Fischer344大鼠脑胶质瘤的疗效及预后.方法 Fischer344大鼠胶质瘤模型建立成功后,随机分为空白对照组、手术组、氩氦冷冻组,每组10只.游标卡尺测量并计算肿瘤体积,观察各组大鼠行为及生存期.结果 空白对照组、手术组和氩氦冷冻组大鼠生存时间分别为(78.5±1.1)d、(171.0±10.8)d和(252.8±5.0)d,差异具有统计学意义(P=0.002).氩氦冷冻组肿瘤体积呈逐渐缩小趋势.结论 氩氦冷冻是治疗胶质瘤有效方法,推测可能与瘤细胞破裂,抗原暴露,而刺激机体产生抗肿瘤的抗体有关.

  4. Density of atoms in Ar*(3p54s) states and gas temperatures in an argon surfatron plasma measured by tunable laser spectroscopy

    Science.gov (United States)

    Hübner, S.; Sadeghi, N.; Carbone, E. A. D.; van der Mullen, J. J. A. M.

    2013-04-01

    This study presents the absolute argon 1 s (in Paschens's notation) densities and the gas temperature, Tg, obtained in a surfatron plasma in the pressure range 0.65recorded with two tunable diode lasers. Tg is deduced from the absorption line shapes when scanning the laser wavelengths. The line profile, which is a Doppler broadening dominated Gaussian at gas pressures of p 10 mbar, for which the pressure broadening can no more be neglected. Tg is in the range of 480-750 K, increasing with pressure and decreasing with the distance from the microwave launcher. Taking into account the line of sight effects of the absorption measurements, a good agreement is found with our previous measurements by Rayleigh scattering of Tg at the tube center. In the studied pressure range, the Ar(4 s) atom densities are in the order of 1016-1018 m-3, increasing towards the end of the plasma column, decreasing with the pressure. In the low pressure side, a broad minimum is found around 10Radiative Model.

  5. Direct solid analysis of powdered tungsten carbide hardmetal precursors by laser-induced argon spark ablation with inductively coupled plasma atomic emission spectrometry.

    Science.gov (United States)

    Holá, Markéta; Kanický, Viktor; Mermet, Jean-Michel; Otruba, Vítezslav

    2003-12-01

    The potential of the laser-induced argon spark atomizer (LINA-Spark atomizer) coupled with ICP-AES as a convenient device for direct analysis of WC/Co powdered precursors of sintered hardmetals was studied. The samples were presented for the ablation as pressed pellets prepared by mixing with powdered silver binder containing GeO2 as internal standard. The pellets were ablated with the aid of a Q-switched Nd:YAG laser (1064 nm) focused 16 mm behind the target surface with a resulting estimated power density of 5 GW cm(-2). Laser ablation ICP-AES signals were studied as a function of ablation time, and the duration of time prior to measurement (pre-ablation time) which was necessary to obtain reliable results was about 40 s. Linear calibration plots were obtained up to 10% (m/m) Ti, 9% Ta and 3.5% Nb both without internal standardization and by using germanium as an added internal standard or tungsten as a contained internal standard. The relative uncertainty at the centroid of the calibration line was in the range from +/- 6% to +/- 11% for Nb, Ta and Ti both with and without internal standardisation by Ge. A higher spread of points about the regression was observed for cobalt for which the relative uncertainty at the centroid was in the range from +/- 9% to +/- 14%. Repeatability of results was improved by the use of both Ge and W internal standards. The lowest determinable quantities calculated for calibration plots were 0.060% Co, 0.010% Nb, 0.16% Ta and 0.030% Ti with internal standardization by Ge. The LA-ICP-AES analyses of real samples led to good agreement with the results obtained by solution-based ICP determination with a relative bias not exceeding 10%. The elimination of the dissolution procedure of powdered tungsten (Nb, Ta, Ti) carbide is the principal advantage of the developed LA-ICP-AES method.

  6. Alternatives to argon for gas stopping volumes in the B194 neutron imager

    Energy Technology Data Exchange (ETDEWEB)

    Bleuel, D. L. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Anderson, S. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Caggiano, J. A. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Hall, J. M. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Johnson, M. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Ratkiewicz, A. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Rusnak, B. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

    2017-05-17

    In a recent experiment at Lawrence Berkeley National Laboratory, the 40Ar(d,p)41Ar excitation function between 3-7 MeV was measured, confirming a previous estimation that there may be an intolerable radiation dose from 41Ar production by slowing to rest 6.74 MeV deuterons in the gas cell of the neutron imaging facility being constructed in B194. Gas alternatives to argon are considered, including helium, nitrogen (N2), neon, sulfur hexafluoride (SF6), krypton, and xenon, as well as high atomic number solid backings such as tantalum.

  7. Multiple ionization of argon by helium ions

    Science.gov (United States)

    Montanari, C. C.; Miraglia, J. E.

    2016-09-01

    We apply the continuum distorted-wave eikonal initial state and the independent electron model to describe the multiple ionization of Ar by He2+ and He+ in the energy range 0.1-10 Mev amu-1. Auger-like post collisional processes are included, which enhance the high energy multiple ionization cross sections via ionization of the inner shells. All Ar electrons (K, L and M-shells) have been included in these calculations. The results agree well with the experimental data at high energies, where the post-collisional ionization is the main contribution. At intermediate impact energies the description is also good though it tends to overestimate the triple and quadruple ionization data at intermediate energies. We analyze this by comparing the present results for He+2 in Ar, with previous ones for He+2 in Ne and Kr. It was found that the theoretical description improves from Ne to Ar and Kr, with the latter being nicely described even at intermediate energies. The present formalism is also tested for Ar inner shell and total ionization cross sections. In all the cases the results above 0.1 MeV amu-1 are quite reasonable, as compared with the experimental data available and with the ECPSSR values.

  8. Fragmentation of phosphorylated and singly charged peptide ions via interaction with metastable atoms.

    Science.gov (United States)

    Berkout, Vadym D; Doroshenko, Vladimir M

    2008-12-01

    Fragmentation of phosphorylated peptide ions via interaction with electronically excited metastable argon atoms was studied in a linear trap - time-of-flight mass spectrometer. Doubly charged ions of phosphorylated peptides from an Enolase digest were produced by electrospray ionization and subjected to a metastable atom beam in the linear trap. The metastable argon atoms were generated using a glow-discharge source. An intensive series of c- and z- ions were observed in all cases, with the phosphorylation group intact. The formation of molecular radical cations with reduced charge indicated that an electron transfer from a highly excited metastable state of argon to the peptide cation occurred. Additionally, singly charged Bradykinin, Substance P and Fibrinopeptide A molecular ions were fragmented via interaction with electronically excited metastable helium atoms. The fragmentation mechanism was different in this case and involved Penning ionization.

  9. Fabrication and characterization of tunnel barriers in a multi-walled carbon nanotube formed by argon atom beam irradiation

    Energy Technology Data Exchange (ETDEWEB)

    Tomizawa, H. [Advanced Device Laboratory, RIKEN, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Department of Applied Physics, Tokyo University of Science, 6-3-1 Niijuku, Katsushika-ku, Tokyo 125-8585 (Japan); Yamaguchi, T., E-mail: tyamag@riken.jp [Advanced Device Laboratory, RIKEN, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Akita, S. [Department of Physics and Electronics, Osaka Prefecture University, 1-1 Gakuen-cho, Nakaku, Sakai, Osaka 599-8531 (Japan); Ishibashi, K. [Advanced Device Laboratory, RIKEN, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Department of Applied Physics, Tokyo University of Science, 6-3-1 Niijuku, Katsushika-ku, Tokyo 125-8585 (Japan); RIKEN Center for Emergent Matter Science (CEMS), 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan)

    2015-07-28

    We have evaluated tunnel barriers formed in multi-walled carbon nanotubes (MWNTs) by an Ar atom beam irradiation method and applied the technique to fabricate coupled double quantum dots. The two-terminal resistance of the individual MWNTs was increased owing to local damage caused by the Ar beam irradiation. The temperature dependence of the current through a single barrier suggested two different contributions to its Arrhenius plot, i.e., formed by direct tunneling through the barrier and by thermal activation over the barrier. The height of the formed barriers was estimated. The fabrication technique was used to produce coupled double quantum dots with serially formed triple barriers on a MWNT. The current measured at 1.5 K as a function of two side-gate voltages resulted in a honeycomb-like charge stability diagram, which confirmed the formation of the double dots. The characteristic parameters of the double quantum dots were calculated, and the feasibility of the technique is discussed.

  10. Ab initio interaction potentials and scattering lengths for ultracold mixtures of metastable helium and alkali-metal atoms

    Science.gov (United States)

    Kedziera, Dariusz; Mentel, Łukasz; Żuchowski, Piotr S.; Knoop, Steven

    2015-06-01

    We have obtained accurate ab initio +4Σ quartet potentials for the diatomic metastable triplet helium+alkali-metal (Li, Na, K, Rb) systems, using all-electron restricted open-shell coupled cluster singles and doubles with noniterative triples corrections CCSD(T) calculations and accurate calculations of the long-range C6 coefficients. These potentials provide accurate ab initio quartet scattering lengths, which for these many-electron systems is possible, because of the small reduced masses and shallow potentials that result in a small amount of bound states. Our results are relevant for ultracold metastable triplet helium+alkali-metal mixture experiments.

  11. Multiconfiguration Dirac-Hartree-Fock energy levels, oscillator strengths, transition probabilities, hyperfine constants and Landé g-factor of intermediate Rydberg series in neutral argon atom

    Science.gov (United States)

    Salah, Wa'el; Hassouneh, Ola

    2017-04-01

    We computed the energy levels, oscillator strengths f_{ij}, the radiative transition rates A_{ij}, the Landé g -factor, the magnetic dipole moment and the electric quadrupole hyperfine constants of the intermediate Rydberg series ns [k]J ( 4 ≤ n ≤ 6), nd [k]J (3 ≤ n ≤ 4), np [k]J (4 ≤ n ≤ 5) relative to the ground state 3p6 1S0 for neutral argon atom spectra. The values are obtained in the framework of the multiconfiguration Dirac-Hartree-Fock (MCDHF) approach. In this approach, Breit interaction, leading quantum electrodynamics (QED) effects and self-energy correction are taken into account. Moreover, these spectroscopic parameters have been calculated for many levels belonging to the configuration 3p54s, 3p55s, 3p56s, 3p53d, 3p54d, 3p54p, 3p55p as well as for transitions between levels 3p54s-3p54p, 3p54p-3p53d, 3p54p-3p55s, 3p55s-3p55p and 3p55p-3p56s. The large majority of the lines from the 4p-5s and 4p-3d, 5s-5p and 5p-6s transition arrays have been observed and the calculations are consistent with the J -file-sum rule. The obtained theoretical values are compared with previous experimental and theoretical data available in the literature. An overall satisfactory agreement is noticed allowing assessing the reliability of our data.

  12. Quantum fluid dynamics based current-density functional study of a helium atom in a strong time-dependent magnetic field

    Science.gov (United States)

    Vikas, Hash(0x125f4490)

    2011-02-01

    Evolution of the helium atom in a strong time-dependent (TD) magnetic field ( B) of strength up to 1011 G is investigated through a quantum fluid dynamics (QFD) based current-density functional theory (CDFT). The TD-QFD-CDFT computations are performed through numerical solution of a single generalized nonlinear Schrödinger equation employing vector exchange-correlation potentials and scalar exchange-correlation density functionals that depend both on the electronic charge-density and the current-density. The results are compared with that obtained from a B-TD-QFD-DFT approach (based on conventional TD-DFT) under similar numerical constraints but employing only scalar exchange-correlation potential dependent on electronic charge-density only. The B-TD-QFD-DFT approach, at a particular TD magnetic field-strength, yields electronic charge- and current-densities as well as exchange-correlation potential resembling with that obtained from the time-independent studies involving static (time-independent) magnetic fields. However, TD-QFD-CDFT electronic charge- and current-densities along with the exchange-correlation potential and energy differ significantly from that obtained using B-TD-QFD-DFT approach, particularly at field-strengths >109 G, representing dynamical effects of a TD field. The work concludes that when a helium atom is subjected to a strong TD magnetic field of order >109 G, the conventional TD-DFT based approach differs "dynamically" from the CDFT based approach under similar computational constraints.

  13. Atomic-scale Modeling of Interactions of Helium, Vacancies and Helium-vacancy Clusters with Screw Dislocations in Alpha-Iron

    Energy Technology Data Exchange (ETDEWEB)

    Heinisch, Howard L.; Gao, Fei; Kurtz, Richard J.

    2010-05-01

    The interactions of He and vacancy defects with <111> screw dislocations in alpha-Fe are modeled using molecular statics, molecular dynamics and transition state energy determinations. The formation energies and binding energies of interstitial He atoms, vacancies and He-vacancy clusters near and within dislocations in alpha-Fe are determined at various locations relative to the dislocation core. Using the dimer transition state method the migration energies and trajectories of the He and vacancy defects near and within the screw dislocation are also determined. Both interstitial He atoms and single vacancies are attracted to and trapped in the dislocation core region, and they both migrate along the dislocation line with a migration energy of about 0.4 eV, which is about half the migration energy of vacancies in the perfect crystal and about five times the migration energy for interstitial He in the perfect crystal. Divacancies and He-divacancy complexes have migration properties within the dislocation core that are similar to those in the perfect crystal, although the stability of these defects within the dislocation may be somewhat less than in the perfect crystal.

  14. Argon-helium cryoablation for prostate cancer:report of 26 cases%氩氦刀低温冷冻治疗前列腺癌:26例报告

    Institute of Scientific and Technical Information of China (English)

    李珲; 胡文勇; 毕泗成; 孙晓俊; 靖万林; 张讯; 崔亮; 李景敏

    2013-01-01

    Objective To evaluate the clinical efficiency of argon-helium cryoablation for prostate cancer. Methods The ENDOCARE cryosurgical system with 2mm Cryoprobes was used to treat the prostate cancer guided by transrectal ultrasound or abdomen ultrasound in 26 patients with a mean age of 73.2 (ranging from 65 to 89) years in our department from 1990 to 2012. Biopsy of the prostate was carried out under the guide of ultrasound at 1 and 3 months after cryotherapy for pathological observation. Results The patients were all followed up for 3 to 24 months. The biopsy results showed that 19 cases were pathologically negative and 7 cases were positive. The obstructions of bladder outlet were all relieved, and hematuria was attenuated or disappeared. Serum prostatic specific antigen (PSA) level was decreased obviously. Bone metastases partially disappeared or shrunk. Bone pain was relieved to some extent. Twenty of them were able to urinate. All patients had their serum levels of PSA lower than 4ng/ml at 3 to 24 months after cryoablation. Conclusion Cryoablation combined with anti-androgen drug has better clinical outcome in the treatment of prostate cancer, with advantages of short hospitalization period, no blood loss, little injury and rapid recovery.%  目的评价氩氦刀低温冷冻治疗前列腺癌的临床效果。方法采用美国ENDOCARE公司制造的CRYDCARE低温手术系统进行手术。26例前列腺癌患者在腰麻或硬膜外麻醉下,经直肠超声或腹部超声术中定位监测,实施前列腺超低温治疗。分别于冷冻治疗术后1个月和3个月时,在直肠超声引导下行前列腺穿刺活检并进行病理检查。结果术后穿刺病理结果显示,肿瘤阴性19例,阳性7例。治疗后排尿梗阻症状均有好转,血尿减轻或消失。26例随访3~24个月,血清前列腺特异性抗原(PSA)明显降低,骨转移灶部分消失或缩小,骨痛缓解。其中20例恢复自行排尿。术后3~24

  15. Effects of autoionization in electron loss from helium-like highly charged ions in collisions with photons and fast atomic particles

    CERN Document Server

    Lyashchenko, K N; Voitkiv, A B

    2016-01-01

    We study theoretically single electron loss from helium-like highly charged ions involving excitation and decay of autoionizing states of the ion. Electron loss is caused by either photo absorption or the interaction with a fast atomic particle (a bare nucleus, a neutral atom, an electron). The interactions with the photon field and the fast particles are taken into account in the first order of perturbation theory. Two initial states of the ion are considered: $1s^2$ and $(1s2s)_{J=0}$. We analyze in detail how the shape of the emission pattern depends on the atomic number $Z_{I}$ of the ion discussing, in particular, the inter-relation between electron loss via photo absorption and due to the impact of atomic particles in collisions at modest relativistic and extreme relativistic energies. According to our results, in electron loss from the $1s^2$ state autoionization may substantially influence the shape of the emission spectra only up to $Z_{I} \\approx 35-40$. A much more prominent role is played by autoi...

  16. Ultra-low-temperature reactions of C({sup 3}P{sub 0}) atoms with benzene molecules in helium droplets

    Energy Technology Data Exchange (ETDEWEB)

    Krasnokutski, Serge A., E-mail: skrasnokutskiy@yahoo.com; Huisken, Friedrich, E-mail: friedrich.huisken@uni-jena.de [Laboratory Astrophysics Group of the Max Planck Institute for Astronomy at the Friedrich Schiller University Jena, Institute of Solid State Physics, Helmholtzweg 3, D-07743 Jena (Germany)

    2014-12-07

    The reaction of carbon atoms with benzene has been investigated in liquid helium droplets at T = 0.37 K. We found an addition of the carbon atom to form an initial intermediate complex followed by a ring opening and the formation of a seven-membered ring. In contrast to a previous gas phase study, the reaction is frozen after these steps and the loss of hydrogen does not occur. A calorimetric technique was applied to monitor the energy balance of the reaction. It was found that more than 267 kJ mol{sup −1} were released in this reaction. This estimation is in line with quantum chemical calculations of the formation energy of a seven-membered carbon ring. It is suggested that reactions of this kind could be responsible for the low abundance of small polycyclic aromatic hydrocarbon molecules in the interstellar medium. We also found the formation of weakly bonded water-carbon adducts, in which the carbon atom is linked to the oxygen atom of the water molecule with a binding energy of about 33.4 kJ mol{sup −1}.

  17. Separation of seven arsenic compounds by high-performance liquid chromatography with on-line detection by hydrogen–argon flame atomic absorption spectrometry and inductively coupled plasma mass spectrometry

    DEFF Research Database (Denmark)

    Hansen, S. H.; Larsen, E. H.; Pritzl, G.

    1992-01-01

    Seven molecular forms of arsenic were separated by anion- and cation-exchange high-performance liquid chromatography (HPLC) with on-line detection by flame atomic absorption spectrometry (FAAS). The interfacing was established by a vented poly(tetrafluoroethylene) capillary tubing connecting...... the HPLC column to the nebulizer of the atomic absorption spectrometer. Arsenite, arsenate, monomethylarsonate (MMA) and dimethylarsinate (DMA) were separated from each other and from the co-injected cationic arsenic compounds, arsenobetaine (AsB), arsenocholine (AsC) and the tetramethylarsonium ion (TMAs......-to-noise ratio of the on-line AAS detector was optimized. This involved the use of the hydrogen-argon-entrained air flame, a slotted tube atom trap in the flame for signal enhancement, electronic noise damping and a high-intensity light source. The detection limits in mu-g cm-3, using 100 mm3 injections...

  18. Separation of seven arsenic compounds by high performance liquid chromatography with on-line detection by hydrogen-argon flame atomic absorption spectrometry and inductively coupled plasma mass spectrometry

    DEFF Research Database (Denmark)

    Hansen, S. H.; Larsen, Erik Huusfeldt; Pritzl, G.

    1992-01-01

    Seven molecular forms of arsenic were separated by anion- and cation-exchange high-performance liquid chromatography (HPLC) with on-line detection by flame atomic absorption spectrometry (FAAS). The interfacing was established by a vented poly(tetrafluoroethylene) capillary tubing connecting......-to-noise ratio of the on-line AAS detector was optimized. This involved the use of the hydrogen-argon-entrained air flame, a slotted tube atom trap in the flame for signal enhancement, electronic noise damping and a high-intensity light source. The detection limits in mu-g cm-3, using 100 mm3 injections...... the HPLC column to the nebulizer of the atomic absorption spectrometer. Arsenite, arsenate, monomethylarsonate (MMA) and dimethylarsinate (DMA) were separated from each other and from the co-injected cationic arsenic compounds, arsenobetaine (AsB), arsenocholine (AsC) and the tetramethylarsonium ion (TMAs...

  19. State-Selective and Total Single-Capture Cross Sections for Fast Collisions of Multiply Charged Ions with Helium Atoms

    Science.gov (United States)

    Mančev, Ivan; Milojević, Nenad; Belkić, Dževad

    2013-11-01

    The four-body boundary corrected first Born approximation (CB1-4B) is used to calculate the single electron capture cross sections for collisions between fully stripped ions (He2+, Be4+, B5+ and C6+) and helium target at intermediate and high impact energies. The main goal of this study is to assess the usefulness of the CB1-4B method at intermediate and high impact energies for these collisions. Detailed comparisons with the measurements are carried out and the obtained theoretical cross sections are in reasonable agreement with the available experimental data.

  20. Ejection of quasi-free electron pairs from the helium atom ground state by single photon absorption

    CERN Document Server

    Schöffler, M S; Waitz, M; Trinter, F; Jahnke, T; Lenz, U; Jones, M; Belkacem, A; Landers, A; Pindzola, M S; Cocke, C L; Colgan, J; Kheifets, A; Bray, I; Schmidt-Böcking, H; Dörner, R; Weber, Th

    2012-01-01

    We investigate single photon double ionization (PDI) of helium at photon energies of 440 and 800 eV. We observe doubly charged ions with close to zero momentum corresponding to electrons emitted back-to-back with equal energy. These slow ions are the unique fingerprint of an elusive quasi-free PDI mechanism predicted by Amusia et al. nearly four decades years ago [J. Phys. B 8, 1248, (1975)] . It results from the non-dipole part of the electromagnetic interaction. Our experimental data are in excellent agreement with calculations performed using the convergent close coupling and time dependent close coupling methods.

  1. Withdrawal of Chinese Physics Letters 28 (2011) 043401 “Measurement of Absolute Atomic Collision Cross Section with Helium Using 87Rb Atoms Confined in Magneto-Optic and Magnetic Traps” by WANG Ji-Cheng et al.

    Institute of Scientific and Technical Information of China (English)

    WANG Ji-Cheng; ZHOU Ke-Ya; WANG Yue-Yuan; LIAO Qing-Hong; LIU Shu-Tian

    2011-01-01

    We announce the withdrawal of the article entitled “Measurement of Absolute Atomic Collision Cross Section with Helium Using 87Rb Atoms Confined in Magneto-Optic and Magnetic Traps”,which was published in Chinese Physics Letters [28(4)(2011)043401].The first author,Jicheng Wang,had participated in related research with Professor Kirk Madison's group at the Department of Physics & Astronomy at the University of British Columbia,Canada from September 2008 to February 2010.Even though consent had been granted for some of the experimental data to be used by Jicheng Wang in his own thesis,its publication had not been authorized.We apologize to Professor K.Madison for the misunderstanding,and to Chinese Physics Letters and the readers of Chinese Physics Letters for any inconvenience this mistake may have caused.%We announce the withdrawal of the article entitled "Measurement of Absolute Atomic Collision Cross Section with Helium Using 87Rb Atoms Confined in Magneto-Optic and Magnetic Traps", which was published in Chinese Physics Letters [28(4) (2011)043401]. The first author, Jicheng Wang, had participated in related research with Professor Kirk Madison's group at the Department of Physics & Astronomy at the University of British Columbia, Canada from September 2008 to February 2010. Even though consent had been granted for some of the experimental data to be used by Jicheng Wang in his own thesis, its publication had not been authorized. We apologize to Professor K. Madison for the misunderstanding, and to Chinese Physics Letters ad the readers of Chinese Physics Letters for any inconvenience this mistake may have caused.

  2. Theoretical research on multiple rescatterings in the process of high-order harmonic generation from a helium atom with a long wavelength

    Science.gov (United States)

    Zhang, Cai-Ping; Pei, Ya-Nan; Xia, Chang-Long; Jia, Xiang-Fu; Miao, Xiang-Yang

    2017-01-01

    The phenomenon of multiple rescatterings in the process of high-order harmonic generation from a helium atom with a long wavelength is investigated by solving the time-dependent Schrödinger equation and the classical equation of motion. The results present the rule of cutoff energies for the multirescattering events. What is more, the physical picture of the multiple rescatterings is built and the physical mechanism is revealed in detail. Further studies show that the multiple rescatterings can be manipulated effectively and the intra-cycle interference of multiple rescatterings is weakened simultaneously when the initial state is prepared in the superposition state. Additionally, the long quantum path is verified to play an important role in the multiple rescattering processes.

  3. Quantum fluid dynamics based current-density functional study of a helium atom in a strong time-dependent magnetic field

    Energy Technology Data Exchange (ETDEWEB)

    Vikas [Quantum Chemistry Group, Department of Chemistry and Centre of Advanced Studies in Chemistry, Panjab University, 160014 Chandigrah (India)

    2011-02-15

    Evolution of the helium atom in a strong time-dependent (TD) magnetic field (B) of strength up to 10{sup 11} G is investigated through a quantum fluid dynamics (QFD) based current-density functional theory (CDFT). The TD-QFD-CDFT computations are performed through numerical solution of a single generalized nonlinear Schroedinger equation employing vector exchange-correlation potentials and scalar exchange-correlation density functionals that depend both on the electronic charge-density and the current-density. The results are compared with that obtained from a B-TD-QFD-DFT approach (based on conventional TD-DFT) under similar numerical constraints but employing only scalar exchange-correlation potential dependent on electronic charge-density only. The B-TD-QFD-DFT approach, at a particular TD magnetic field-strength, yields electronic charge- and current-densities as well as exchange-correlation potential resembling with that obtained from the time-independent studies involving static (time-independent) magnetic fields. However, TD-QFD-CDFT electronic charge- and current-densities along with the exchange-correlation potential and energy differ significantly from that obtained using B-TD-QFD-DFT approach, particularly at field-strengths >10{sup 9} G, representing dynamical effects of a TD field. The work concludes that when a helium atom is subjected to a strong TD magnetic field of order >10{sup 9} G, the conventional TD-DFT based approach differs 'dynamically' from the CDFT based approach under similar computational constraints. (author)

  4. Enhanced creation of dispersive monolayer phonons in Xe/Pt(111) by inelastic helium atom scattering at low energies

    DEFF Research Database (Denmark)

    Hansen, Flemming Yssing; Bruch, Ludwig Walter

    2007-01-01

    Conditions likely to lead to enhanced inelastic atomic scattering that creates shear horizontal (SH) and longitudinal acoustic (LA) monolayer phonons are identified, specifically examining the inelastic scattering of He-4 atoms by a monolayer solid of Xe/Pt(111) at incident energies of 2-25 meV. ...

  5. Study on the clinical efficacy of CT guided percutaneous argon helium knife for the treatment of metastatic bone tumor%CT 引导下经皮穿刺氩氦刀冷冻技术对转移性骨肿瘤的临床疗效观察与研究

    Institute of Scientific and Technical Information of China (English)

    赵朝阳; 邓少杰; 叶军; 张在恒; 刘文华

    2016-01-01

    目的:观察研究 CT 引导下经皮穿刺氩氦刀冷冻技术对转移性骨肿瘤的临床疗效。方法选取我院98例转移性骨肿瘤患者,回顾性分析上述患者临床治疗效果,比较患者治疗前后视觉模拟评分(VAS)及卡氏功能状态评分标准(KPS)评分变化,以及术后不良反应及并发症发生情况,总结 CT 引导下经皮穿刺氩氦刀冷冻技术优缺点。结果98例转移性骨肿瘤患者,均穿刺获得满意标本,一次性成功。其中活检穿刺发现肺癌骨转移人数最多,共72例,占73.47%,其次为肝癌骨转移,共19例,占19.39%,恶性黑色素瘤7例,占7.14%。本组98例 CT 引导下经皮穿刺氩氦刀冷冻治疗后并发症发生率为30.06%(30/98),其中血压升高严重者为3例,占3.06%,皮肤严重冻伤者1例,占1.02%。98例患者治疗后 VAS 和 KPS 评分较治疗前有显著下降(P <0.01)。结论 CT 引导下经皮穿刺氩氦刀冷冻技术不仅可以达到与常规方法治疗的准确率,且对恶性病灶的敏感度高,氩氦刀冷冻组织时定位准确,创口小,成功度较高,在保留骨诱导活性和保存肢体的前提下进行治疗。对转移性骨肿瘤患者进行 CT 引导下经皮穿刺氩氦刀冷冻治疗在降低局部复发率,保留骨诱导活性以及改善关节功能方面的临床应用前景广阔。%Objective To observe the clinical effect of CT guided percutaneous argon helium knife in the treatment of metastatic bone tumor.Methods Ninety-eight patients with metastatic bone tumor in our hospital were analyzed retrospectively.The clinical treatment and changes of VAS and KPS score were studied.Results 98 cases of patients with metastatic bone tumor were successfully sampled.Biopsy puncture showed that the largest number of lung cancer bone metastasis is 72,accounting for 73.47%;followed by 19 cases of bone metastasis of liver cancer,accounting for

  6. Molecular Dynamics Simulations of Helium Behaviour in Titanium Crystals

    Institute of Scientific and Technical Information of China (English)

    SUN Tie-Ying; LONG Xing-Gui; WANG Jun; HOU Qing; WU Zhong-Cheng; PENG Shu-Ming; LUO Shun-Zhong

    2008-01-01

    Molecular dynamics simulations are performed to investigate the behaviour of helium atoms in titanium at a temperature of 300 K.The nucleation and growth of helium bubble has been simulated up to 50 helium atoms.The approach to simulate the bubble growth is to add helium atoms one by one to the bubble and let the system evolve.The titanium cohesion is based on the tight binding scheme derived from the embedded atom method,and the helium-titanium interaction is characterized by fitted potential in the form of a Lennard-Jones function.The pressure in small helium bubbles is approximately calculated.The simulation results show that the pressure will decrease with the increasing bubble size,while increase with the increasing helium atoms.An analytic function about the quantitative relationship of the pressure with the bubble size and number of helium atoms is also fitted.

  7. Alkali-helium snowball complexes formed on helium nanodroplets.

    Science.gov (United States)

    Müller, S; Mudrich, M; Stienkemeier, F

    2009-07-28

    We systematically investigate the formation and stability of snowballs formed by femtosecond photoionization of small alkali clusters bound to helium nanodroplets. For all studied alkali species Ak = (Na,K,Rb,Cs) we observe the formation of snowballs Ak(+)He(N) when multiply doping the droplets. Fragmentation of clusters Ak(N) upon ionization appears to enhance snowball formation. In the case of Na and Cs we also detect snowballs Ak(2) (+)He(N) formed around Ak dimer ions. While the snowball progression for Na and K is limited to less than 11 helium atoms, the heavier atoms Rb and Cs feature wide distributions at least up to Ak(+)He(41). Characteristic steps in the mass spectra of Cs-doped helium droplets are found at positions consistent with predictions on the closure of the first shell of helium atoms around the Ak(+) ion based on variational Monte Carlo simulations.

  8. Liquid helium

    CERN Document Server

    Atkins, K R

    1959-01-01

    Originally published in 1959 as part of the Cambridge Monographs on Physics series, this book addresses liquid helium from the dual perspectives of statistical mechanics and hydrodynamics. Atkins looks at both Helium Three and Helium Four, as well as the properties of a combination of the two isotopes. This book will be of value to anyone with an interest in the history of science and the study of one of the universe's most fundamental elements.

  9. Charging dynamics of dopants in helium nanoplasmas

    DEFF Research Database (Denmark)

    Heidenreich, Andreas; Grüner, Barbara; Schomas, Dominik

    2017-01-01

    We present a combined experimental and theoretical study of the charging dynamics of helium nanodroplets doped with atoms of different species and irradiated by intense near-infrared laser pulses (≤1015 W cm−2). In particular, we elucidate the interplay of dopant ionization inducing the ignition...... of a helium nanoplasma, and the charging of the dopant atoms driven by the ionized helium host. Most efficient nanoplasma ignition and charging is found when doping helium droplets with xenon atoms, in which case high charge states of both helium (He2+) and of xenon (Xe21+) are detected. In contrast, only low...... charge states of helium and dopants are measured when doping with potassium and calcium atoms. Classical molecular dynamics simulations which include focal averaging generally reproduce the experimental results and provide detailed insights into the correlated charging dynamics of guest and host clusters....

  10. Effect of dislocations on helium retention in deformed pure iron

    Science.gov (United States)

    Gong, Y. H.; Cao, X. Z.; Jin, S. X.; Lu, E. Y.; Hu, Y. C.; Zhu, T.; Kuang, P.; Xu, Q.; Wang, B. Y.

    2016-12-01

    The effects of dislocations created by deformation on helium retention in pure iron, including the helium atoms diffusion along the dislocation line and desorption from dislocation trapping sites, were investigated. The dislocation defect was introduced in specimens by cold-rolling, and then 5 keV helium ions were implanted into the deformed specimens. Slow positron beam technology and thermal desorption spectroscopy were used to investigate the evolution of dislocation defects and the desorption behavior of helium atoms under influence of dislocation. The behaviors of S-E, W-E and S-W plots indicate clearly that lots of helium atoms remain in the deformed specimen and helium atoms combining with dislocation change the distribution of electron density. The helium desorption plot indicates that dislocation accelerates helium desorption at 293 K-600 K and facilitates helium dissociation from HenVm (n/m = 1.8) cluster.

  11. Quantum-state-controlled Penning-ionization reactions between ultracold alkali-metal and metastable helium atoms

    Science.gov (United States)

    Flores, A. S.; Vassen, W.; Knoop, S.

    2016-11-01

    In an ultracold, optically trapped mixture of 87Rb and metastable triplet 4He atoms we have studied trap loss for different spin-state combinations, for which interspecies Penning ionization is the main two-body loss process. We observe long trapping lifetimes for the purely quartet spin-state combination, indicating strong suppression of Penning-ionization loss by at least two orders of magnitude. For the other spin mixtures we observe short lifetimes that depend linearly on the doublet character of the entrance channel. We compare the extracted loss rate coefficient with recent predictions of multichannel quantum-defect theory for reactive collisions involving a strong exothermic loss channel and find near-universal loss for doublet scattering. Our work demonstrates control of Penning-ionization reactive collisions by internal atomic state preparation.

  12. Current mapping of low-energy (120 eV) helium and hydrogen irradiated tungsten by conductive atomic force microscopy

    Science.gov (United States)

    Fan, Hongyu; Endo, Takashi; Bi, Zhenghua; Yan, Weibin; Ohnuki, Somei; Yang, Qi; Ni, Weiyuan; Liu, Dongping

    2017-04-01

    Both conductive atomic force microscopy (CAFM) and transmission electron microscopy have been used to characterize the defects or He bubbles in low-energy (120 eV) H and He irradiated tungsten (W). By a comparative study, we find that the current mapping from CAFM is very sensitive in the detection of nanometer-sized defects in low-energy H and He irradiated W. Our calculation confirms that the resistance change in H and He irradiated W is strongly affected by the distance between atomic force microscopy tip and defects/He bubbles. CAFM can accurately detect defects/He bubbles in the W surface layer, however, it is infeasible to measure them in the deep layer (>20 nm), especially due to the existence of defects in the surface layer.

  13. Theoretical state-selective and total cross sections for electron capture from helium atoms by fully stripped ions

    Science.gov (United States)

    Mančev, I.; Milojević, N.; Belkić, Dž.

    2015-03-01

    The four-body boundary-corrected first Born (CB1-4B) approximation is used to compute cross sections for single electron capture from helium targets by fully stripped ions. The projectile ions are H+, He2+, Li3+, Be4+, B5+, C6+, N7+, O8+, and F9+. An extensive list of theoretical state-to-state cross sections in these collisions at energies ranging from 20 to 10 000 keV/amu is given. This list includes the state-selective cross sections Qnlm for each individual triple of the usual quantum numbers { n , l , m } of the final hydrogen-like states alongside Qnl and Qn for the pertinent sub-shells and shells where the respective summations over m and { l , m } have been carried out. The maximal value of the principal quantum number n was chosen to vary from 4 (H+) to 10 (F9+) so as to satisfy the condition n ≥ZP, where ZP is the nuclear charge of the projectile. Usually, the largest cross sections stem from those values of n that match the projectile charge (n =ZP) . The total cross sections for capture summed over all the quantum numbers { n , l , m } are also tabulated. The overall goal of this study is to fill in lacunae in the existing databases of charge exchange cross sections that are needed in several inter-disciplinary fields. For example, in particle transport physics, which is of utmost importance in such emerging branches as hadron therapy, these cross sections constitute a part of the multifaceted input data for stochastic simulations of energy losses of multiply charged ions in matter, including tissue. Other significant uses of the present data are anticipated in charge exchange diagnostics within thermonuclear research project as well as in applications covering the relevant parts of plasma physics and astrophysics.

  14. Measurement of OH, NO, O and N atoms in helium plasma jet for ROS/RNS controlled biomedical processes

    Science.gov (United States)

    Yonemori, Seiya; Kamakura, Taku; Ono, Ryo

    2014-10-01

    Atmospheric-pressure plasmas are of emerging interest for new plasma applications such as cancer treatment, cell activation and sterilization. In those biomedical processes, reactive oxygen/nitrogen species (ROS/RNS) are said that they play significant role. It is though that active species give oxidative stress and induce biomedical reactions. In this study, we measured OH, NO, O and N atoms using laser induced fluorescence (LIF) measurement and found that voltage polarity affect particular ROS. When negative high voltage was applied to the plasma jet, O atom density was tripled compared to the case of positive applied voltage. In that case, O atom density was around 3 × 1015 [cm-3] at maximum. In contrast, OH and NO density did not change their density depending on the polarity of applied voltage, measured as in order of 1013 and 1014 [cm-3] at maximum, respectively. From ICCD imaging measurement, it could be seen that negative high voltage enhanced secondary emission in plasma bullet propagation and it can affect the effective production of particular ROS. Since ROS/RNS dose can be a quantitative criterion to control plasma biomedical application, those measurement results is able to be applied for in vivo and in vitro plasma biomedical experiments. This study is supported by the Grant-in-Aid for Science Research by the Ministry of Education, Culture, Sport, Science and Technology.

  15. Helium cryogenics

    CERN Document Server

    Van Sciver, Steven W

    2012-01-01

    Twenty five years have elapsed since the original publication of Helium Cryogenics. During this time, a considerable amount of research and development involving helium fluids has been carried out culminating in several large-scale projects. Furthermore, the field has matured through these efforts so that there is now a broad engineering base to assist the development of future projects. Helium Cryogenics, 2nd edition brings these advances in helium cryogenics together in an updated form. As in the original edition, the author's approach is to survey the field of cryogenics with emphasis on helium fluids. This approach is more specialized and fundamental than that contained in other cryogenics books, which treat the associated range of cryogenic fluids. As a result, the level of treatment is more advanced and assumes a certain knowledge of fundamental engineering and physics principles, including some quantum mechanics. The goal throughout the work is to bridge the gap between the physics and engineering aspe...

  16. A simple design for a helium scattering apparatus

    Science.gov (United States)

    Maier, F.; Kneitz, S.; Koschel, H.; Steinrück, H.-P.

    1997-04-01

    We have designed a simple helium scattering apparatus for gas-surface scattering experiments. The effusive source is a glass multicapillary array, operated at large Knudsen numbers which produces a highly collimated thermal He beam (FWHM ≈ 3°) with a Maxwellian velocity distribution. The detector is a Bayard Alpert ionization gauge, mounted in a tube that is separated from the main UHV chamber via a second multicapillary array. This setup allows one to select only those He atoms that are reflected by the sample in the specular direction and thus to measure the reflectivity of the surface. Examples of its performance are presented for the adsorption of CO on Ru(001), and for thermal annealing of a Ru(001) surface sputtered with argon ions at different energies.

  17. Argon Collection And Purification For Proliferation Detection

    Energy Technology Data Exchange (ETDEWEB)

    Achey, R. [Savannah River Site (SRS), Aiken, SC (United States). Savannah River National Lab. (SRNL); Hunter, D. [Savannah River Site (SRS), Aiken, SC (United States). Savannah River National Lab. (SRNL)

    2015-10-09

    In order to determine whether a seismic event was a declared/undeclared underground nuclear weapon test, environmental samples must be taken and analyzed for signatures that are unique to a nuclear explosion. These signatures are either particles or gases. Particle samples are routinely taken and analyzed under the Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO) verification regime as well as by individual countries. Gas samples are analyzed for signature gases, especially radioactive xenon. Underground nuclear tests also produce radioactive argon, but that signature is not well monitored. A radioactive argon signature, along with other signatures, can more conclusively determine whether an event was a nuclear test. This project has developed capabilities for collecting and purifying argon samples for ultra-low-background proportional counting. SRNL has developed a continuous gas enrichment system that produces an output stream containing 97% argon from whole air using adsorbent separation technology (the flow diagram for the system is shown in the figure). The vacuum swing adsorption (VSA) enrichment system is easily scalable to produce ten liters or more of 97% argon within twelve hours. A gas chromatographic separation using a column of modified hydrogen mordenite molecular sieve has been developed that can further purify the sample to better than 99% purity after separation from the helium carrier gas. The combination of these concentration and purification systems has the capability of being used for a field-deployable system for collecting argon samples suitable for ultra-low-background proportional counting for detecting nuclear detonations under the On-Site Inspection program of the CTBTO verification regime. The technology also has applications for the bulk argon separation from air for industrial purposes such as the semi-conductor industry.

  18. Opacity of Shock-Generated Argon Plasmas

    Institute of Scientific and Technical Information of China (English)

    王藩侯; 陈敬平; 周显明; 李西军; 经福谦; 孟续军; 孙永盛

    2001-01-01

    Argon plasmas with uniform density and temperature are generated by a planar shock wave through argon gas. The opacities of argon plasma, covering the thermodynamic states at temperatures of 1.4-2.2eV and in densities of 0.0083- 0.015 g/cm3, are investigated by measuring the emitted radiance versus time at several visible wavelengths. Comparison of the measured opacities with those calculated demonstrates that the average atom model can be used well to describe the essential transport behaviour of photons in argon plasma under the abovementioned thermodynamic condition. A simplified and self-consistent method to deduce the reflectivity R(λ) at the baseplate surface is applied. It demonstrates that the values of R(λ) are all around 0.4 in the experiments, which are basically in agreement with those given by Erskine previously (1994 J. Quant. Spectrosc. Radiat.Transfer 51 97).

  19. Critical Landau velocity in helium nanodroplets.

    Science.gov (United States)

    Brauer, Nils B; Smolarek, Szymon; Loginov, Evgeniy; Mateo, David; Hernando, Alberto; Pi, Marti; Barranco, Manuel; Buma, Wybren J; Drabbels, Marcel

    2013-10-11

    The best-known property of superfluid helium is the vanishing viscosity that objects experience while moving through the liquid with speeds below the so-called critical Landau velocity. This critical velocity is generally considered a macroscopic property as it is related to the collective excitations of the helium atoms in the liquid. In the present work we determine to what extent this concept can still be applied to nanometer-scale, finite size helium systems. To this end, atoms and molecules embedded in helium nanodroplets of various sizes are accelerated out of the droplets by means of optical excitation, and the speed distributions of the ejected particles are determined. The measurements reveal the existence of a critical velocity in these systems, even for nanodroplets consisting of only a thousand helium atoms. Accompanying theoretical simulations based on a time-dependent density functional description of the helium confirm and further elucidate this experimental finding.

  20. Characterization of the Plasma Edge for Technique of Atomic Helium Beam in the CIEMAT Fusion Device; Caracterizacion del Borde del Plasma del Dispositivo de Fusion TJ-II del CIEMAT mediante el Diagnostico del Haz Supersonico de Helio

    Energy Technology Data Exchange (ETDEWEB)

    Hidalgo, A.

    2003-07-01

    In this report, the measurement of Electron Temperature and Density in the Boundary Plasma of TJ-II with a Supersonic Helium Beam Diagnostic and work devoted to the upgrading of this technique are described. Also, simulations of Laser Induced Fluorescence (LIF) studies of level populations of electronically excited He atoms are shown. This last technique is now being installed in the CIEMAT fusion device. (Author ) 36 refs.

  1. New x-ray measurements in Helium-like Atoms increase discrepancy between experiment and theoretical QED

    CERN Document Server

    Chantler, Christopher T; Gillaspy, John D; Hudson, Lawrence T; Smale, Lucas F; Henins, Albert; Kimpton, Justin A; Takacs, Endre

    2014-01-01

    A recent 15 parts-per-million (ppm) experiment on muonic hydrogen found a major discrepancy with QED and independent nuclear size determinations. Here we find a significant discrepancy in a different type of exotic atom, a medium-Z nucleus with two electrons. Investigation of the data collected is able to discriminate between available QED formulations and reveals a pattern of discrepancy of almost 6 standard errors of experimental results from the most recent theoretical predictions with a functional dependence proportional to Z^n where n=4. In both the muonic and highly charged systems, the sign of the discrepancy is the same, with the measured transition energy higher than predicted. Some consequences are possible or probable, and some are more speculative. This may give insight into effective nuclear radii, the Rydberg, the fine-structure constant or unexpectedly large QED terms.

  2. The stereo-dynamics of collisional autoionization of ammonia by helium and neon metastable excited atoms through molecular beam experiments

    Energy Technology Data Exchange (ETDEWEB)

    Falcinelli, Stefano, E-mail: stefano.falcinelli@unipg.it; Vecchiocattivi, Franco [Department of Civil and Environmental Engineering, University of Perugia, Via G. Duranti 93, 06125 Perugia (Italy); Bartocci, Alessio; Cavalli, Simonetta; Pirani, Fernando [Department of Chemistry, Biology, and Biotechnology, University of Perugia, Via Elce di sotto 8, 06123 Perugia (Italy)

    2015-10-28

    A combined analysis of both new (energy spectra of emitted electrons) and previously published (ionization cross sections) experimental data, measured under the same conditions and concerning electronically excited lighter noble gas –NH{sub 3} collisional autoionization processes, is carried out. Such an analysis, performed by exploiting a formulation of the full potential energy surface both in the real and imaginary parts, provides direct information on energetics, structure, and lifetime of the intermediate collision complex over all the configuration space. The marked anisotropy in the attraction of the real part, driving the approach of reagents, and the selective role of the imaginary component, associated to the charge transfer coupling between entrance and exit channels, suggests that reactive events occur almost exclusively in the molecular hemisphere containing the nitrogen lone pair. Crucial details on the stereo-dynamics of elementary collisional autoionization processes are then obtained, in which the open shell nature of the disclosed ionic core of metastable atom plays a crucial role. The same analysis also suggests that the strength of the attraction and the anisotropy of the interaction increases regularly along the series Ne{sup *}({sup 3}P), He{sup *}({sup 3}S), He{sup *}({sup 1}S)–NH{sub 3}. These findings can be ascribed to the strong rise of the metastable atom electronic polarizability (deformability) along the series. The obtained results can stimulate state of the art ab initio calculations focused on specific features of the transition state (energetics, structure, lifetime, etc.) which can be crucial for a further improvement of the adopted treatment and to better understand the nature of the leading interaction components which are the same responsible for the formation of the intermolecular halogen and hydrogen bond.

  3. The stereo-dynamics of collisional autoionization of ammonia by helium and neon metastable excited atoms through molecular beam experiments.

    Science.gov (United States)

    Falcinelli, Stefano; Bartocci, Alessio; Cavalli, Simonetta; Pirani, Fernando; Vecchiocattivi, Franco

    2015-10-28

    A combined analysis of both new (energy spectra of emitted electrons) and previously published (ionization cross sections) experimental data, measured under the same conditions and concerning electronically excited lighter noble gas -NH3 collisional autoionization processes, is carried out. Such an analysis, performed by exploiting a formulation of the full potential energy surface both in the real and imaginary parts, provides direct information on energetics, structure, and lifetime of the intermediate collision complex over all the configuration space. The marked anisotropy in the attraction of the real part, driving the approach of reagents, and the selective role of the imaginary component, associated to the charge transfer coupling between entrance and exit channels, suggests that reactive events occur almost exclusively in the molecular hemisphere containing the nitrogen lone pair. Crucial details on the stereo-dynamics of elementary collisional autoionization processes are then obtained, in which the open shell nature of the disclosed ionic core of metastable atom plays a crucial role. The same analysis also suggests that the strength of the attraction and the anisotropy of the interaction increases regularly along the series Ne*((3)P), He*((3)S), He*((1)S)-NH3. These findings can be ascribed to the strong rise of the metastable atom electronic polarizability (deformability) along the series. The obtained results can stimulate state of the art ab initio calculations focused on specific features of the transition state (energetics, structure, lifetime, etc.) which can be crucial for a further improvement of the adopted treatment and to better understand the nature of the leading interaction components which are the same responsible for the formation of the intermolecular halogen and hydrogen bond.

  4. Effect of additive oxygen gas on cellular response of lung cancer cells induced by atmospheric pressure helium plasma jet.

    Science.gov (United States)

    Joh, Hea Min; Choi, Ji Ye; Kim, Sun Ja; Chung, T H; Kang, Tae-Hong

    2014-10-16

    The atmospheric pressure helium plasma jet driven by pulsed dc voltage was utilized to treat human lung cancer cells in vitro. The properties of plasma plume were adjusted by the injection type and flow rate of additive oxygen gas in atmospheric pressure helium plasma jet. The plasma characteristics such as plume length, electric current and optical emission spectra (OES) were measured at different flow rates of additive oxygen to helium. The plasma plume length and total current decreased with an increase in the additive oxygen flow rate. The electron excitation temperature estimated by the Boltzmann plot from several excited helium emission lines increased slightly with the additive oxygen flow. The oxygen atom density in the gas phase estimated by actinometry utilizing argon was observed to increase with the additive oxygen flow. The concentration of intracellular reactive oxygen species (ROS) measured by fluorescence assay was found to be not exactly proportional to that of extracellular ROS (measured by OES), but both correlated considerably. It was also observed that the expression levels of p53 and the phospho-p53 were enhanced in the presence of additive oxygen flow compared with those from the pure helium plasma treatment.

  5. Estimation Using an Enhancement Factor on Non Local Thermodynamic Equilibrium Behavior of High-lying Energy Levels of Neutral Atom in Argon Radio-Frequency Inductively-Coupled Plasma.

    Science.gov (United States)

    Wagatsuma, Kazuaki; Satoh, Kozue

    2016-01-01

    This paper describes a plasma-diagnostic method using an enhancement factor on the Boltzmann distribution among emission lines of iron atom in an argon radio-frequency inductively-coupled plasma (ICP). It indicated that Boltzmann plots of the atomic lines having lower excitation energies (3.4 to 4.8 eV) were well fitted on a straight line while those having more than 5.5 eV deviated upwards from a linear relationship. This observation could be explained by the fact that ICP is not in a complete thermodynamic equilibrium between direct excitation to energy levels of iron atom, ionization of iron atom, and radiative decay processes to the ground state. Especially, the recombination of iron ion with captured electron should accompany cascade de-excitations between closely-spaced excited levels just below the ionization limit, the rates of which become slower as a whole; as a result, these high-lying levels might be more populated than the low-lying levels as if a different LTE condition coexists on the high energy side. This overpopulation could be quantitatively estimated using an enhancement factor (EF), which was a ratio of the observed intensity to the expected value extrapolated from the normal distribution on the low energy side. The EFs were generally small (less than 3); therefore, the cascade de-excitation process would slightly contribute to the population of these excited levels. It could be considered from variations of the EF that the overpopulation proceeded to a larger extent at lower radio-frequency forward powers, at higher flow rates of the carrier gas, or at higher observation heights. The reason for this is that the kinetic energy of energetic particles, such as electrons, becomes reduced under all of these plasma conditions, thus enabling the high-lying levels to be more populated by cascade de-excitation processes from iron ion rather than by collisional excitation processes with the energetic particles. A similar Boltzmann analysis using the EF

  6. Discovery of underground argon with low level of radioactive 39Ar and possible applications to WIMP dark matter detectors

    CERN Document Server

    Galbiati, C

    2007-01-01

    We report on the first measurement of 39Ar in argon from underground natural gas reservoirs. The gas stored in the US National Helium Reserve was found to contain a low level of 39Ar. The ratio of 39Ar to stable argon was found to be <=4x10-17 (84% C.L.), less than 5% the value in atmospheric argon (39Ar/Ar=8x10-16). The total quantity of argon currently stored in the National Helium Reserve is estimated at 1000 tons. 39Ar represents one of the most important backgrounds in argon detectors for WIMP dark matter searches. The findings reported demonstrate the possibility of constructing large multi-ton argon detectors with low radioactivity suitable for WIMP dark matter searches.

  7. Atoms

    Institute of Scientific and Technical Information of China (English)

    刘洪毓

    2007-01-01

    Atoms(原子)are all around us.They are something like the bricks (砖块)of which everything is made. The size of an atom is very,very small.In just one grain of salt are held millions of atoms. Atoms are very important.The way one object acts depends on what

  8. Theoretical and experimental investigation of (e,2e) ionization of argon 3p in asymmetric kinematics at intermediate energy

    Science.gov (United States)

    Amami, Sadek; Ulu, Melike; Ozer, Zehra Nur; Yavuz, Murat; Kazgoz, Suay; Dogan, Mevlut; Zatsarinny, Oleg; Bartschat, Klaus; Madison, Don

    2014-07-01

    The field of electron-impact ionization of atoms, or (e,2e), has provided significant detailed information about the physics of collisions. For ionization of hydrogen and helium, essentially exact numerical methods have been developed which can correctly predict what will happen. For larger atoms, we do not have theories of comparable accuracy. Considerable attention has been given to ionization of inert gases and, of the inert gases, argon seems to be the most difficult target for theory. There have been several studies comparing experiment and perturbative theoretical approaches over the last few decades, and generally qualitative but not quantitative agreement is found for intermediate energy incident electrons. Recently a nonperturbative method, the B-spline R-matrix (BSR) method, was introduced which appears to be very promising for ionization of heavier atoms. We have recently performed an experimental and theoretical investigation for ionization of argon, and we found that, although the BSR gave reasonably good agreement with experiment, there were also some cases of significant disagreement. The previous study was performed for 200-eV incident electrons and ejected electron energies of 15 and 20 eV. The purpose of the present work is to extend this study to a much larger range of ejected electron energies (15-50 eV) to see if theory gets better with increasing energy as would be expected for a perturbative calculation. The experimental results are compared with both the BSR and two different perturbative calculations.

  9. Excitation and ionization of hydrogen and helium atoms by femtosecond laser pulses: theoretical approach by Coulomb-Volkov states; Excitation et ionisation des atomes d'hydrogene et d'helium par des impulsions laser femtosecondes: approche theorique par des etats de Coulomb-Volkov

    Energy Technology Data Exchange (ETDEWEB)

    Guichard, R

    2007-12-15

    We present a theoretical approach using Coulomb-Volkov states that appears useful for the study of atomic multi-photonic processes induced by intense XUV femtosecond laser pulses. It predicts hydrogen ionization spectra when it is irradiated by laser pulses in perturbations conditions. Three ways have been investigated. Extension to strong fields when {Dirac_h}{omega} > I{sub p}: it requires to include the hydrogen ground state population, introducing it in standard Coulomb-Volkov amplitude leads to saturated multi-photonic ionization. Extension to multi-photonic transitions with {Dirac_h}{omega} < I{sub p}: new quantum paths are open by the possibility to excite the lower hydrogen bound states. Multiphoton excitation of these states is investigated using a Coulomb-Volkov approach. Extension to helium: two-photon double ionization study shows the influence of electronic correlations in both ground and final state. Huge quantity of information such as angular and energetic distributions as well as total cross sections is available. (author)

  10. Charging dynamics of dopants in helium nanoplasmas

    OpenAIRE

    Heidenreich, Andreas; Grüner, Barbara; Schomas, Dominik; Stienkemeier, Frank; Krishnan, Siva Rama; Mudrich, Marcel

    2016-01-01

    We present a combined experimental and theoretical study of the charging dynamics of helium nanodroplets doped with atoms of different species and irradiated by intense near-infrared (NIR) laser pulses (

  11. Effect of oxygen atoms dissociated by non-equilibrium plasma on flame of methane oxygen and argon pre-mixture gas

    Science.gov (United States)

    Akashi, Haruaki; Yoshinaga, Tomokazu; Sasaki, Koichi

    2014-10-01

    For more efficient way of combustion, plasma-assisted combustion has been investigated by many researchers. But it is very difficult to clarify the effect of plasma even on the flame of methane. Because there are many complex chemical reactions in combustion system. Sasaki et al. has reported that the flame length of methane and air premixed burner shortened by irradiating microwave power. They also measured emission from Second Positive Band System of nitrogen during the irradiation. The emission indicates existence of high energy electrons which are accelerated by the microwave. The high energy electrons also dissociate oxygen molecules easily and oxygen atom would have some effects on the flame. But the dissociation ratio of oxygen molecules by the non-equilibrium plasma is significantly low, compared to that in the combustion reaction. To clarify the effect of dissociated oxygen atoms on the flame, dependence of dissociation ratio of oxygen on the flame has been examined using CHEMKIN. It is found that in the case of low dissociation ratio of 10-6, the ignition of the flame becomes slightly earlier. It is also found that in the case of high dissociation ratio of 10-3, the ignition time becomes significantly earlier by almost half. This work was supported by KAKENHI (22340170).

  12. Dispersion forces between noble gas atoms

    NARCIS (Netherlands)

    Lekkerkerker, H.N.W.; Luyckx, R.; Coulon, P.

    1978-01-01

    The coefficients of the R-6, R -8, and R-10 terms in the series representation of the dispersion interaction between helium, neon, and argon at distance R are calculated using an elementary variation method.

  13. 冷冻消融序贯化疗治疗晚期非小细胞肺癌的疗效观察%Clinical efficacy of argon- helium knife cryotherapy followed by chemotherapy for advanced non- small cell lung cancer

    Institute of Scientific and Technical Information of China (English)

    钱建新; 顾小强; 焦晓栋; 王湛; 武清

    2014-01-01

    目的:探讨氩氦刀冷冻消融序贯化疗治疗晚期非小细胞肺癌(NSCLC)的近期疗效以及对远期生存的影响。方法回顾61例行氩氦刀冷冻消融序贯化疗以及同期52例单纯接受化疗的Ⅲb 或Ⅳ期 NSCLC 患者。采用疼痛数字分级法(NRS)行疼痛评估,FACT- G 量表评估生活质量(QOL)。按 RECIST实体瘤疗效评价标准评价疗效,随访患者生存时间。结果①26例患者术前伴有局部疼痛,冷冻术后疼痛有不同程度的缓解。61例患者冷冻术后生活质量 FACT- G 各维度均有不同程度的改善。②与同期单纯化疗的患者比较,冷冻消融序贯化疗组肿瘤缓解率较高(34.4%比15.4%,P <0.05)。③冷冻消融序贯化疗与单纯化疗患者的中位生存时间分别为12.9个月和9.5个月,1年生存率分别为53.6%和35.4%。两组间差异有统计学意义(P <0.01)。结论氩氦刀冷冻消融为一安全、有效的肿瘤局部治疗手段,可迅速降低肿瘤负荷,缓解患者疼痛,改善生活质量。 CT 引导下经皮穿刺氩氦刀冷冻消融治疗肺癌可取得较好疗效,尤其对不能根治切除或不能耐受手术的晚期 NSCLC 患者,冷冻消融后序贯化疗的疗效优于单纯化疗,可提高患者的生存率。%Objective To explore the short- term efficacy of argon- helium knife cryotherapy followed by chemotherapy in treating advanced non- small cell lung cancer (NSCLC) and to investigate its effect on the long- term survival. Methods During the period from March 2005 to March 2008, a total of 61 patients withⅢb or Ⅳ stage NSCLC received argon- helium knife cryotherapy followed by chemotherapy (study group), and other 52 patients with Ⅲb or Ⅳ stage NSCLC were treated with chemotherapy only (control group). The clinical data were retrospectively analyzed. The pain was evaluated by numeric rating scale (NRS) and the quality of life (QOL) was assessed by

  14. Pressure broadening of acetylene rotational Raman lines by argon

    OpenAIRE

    Ceruti, M; Frenkel, D.; Mctaque, J.P.

    1980-01-01

    The anisotropic interaction between acetylene and argon has been studied by observing the density dependence of the acetylene pure rotational Raman line broadening. The observed cross sections are approximately twice that predicted from the known polarizabilities and acetylene molecular quadrupole moment. An empirical atom-atom anisotropic potential adequately parametrizes the results.

  15. Coherent and non coherent atom optics experiment with an ultra-narrow beam of metastable rare gas atoms; Experiences d'optique atomique coherente ou non avec un jet superfin d'atomes metastables de gaz rares

    Energy Technology Data Exchange (ETDEWEB)

    Grucker, J

    2007-12-15

    In this thesis, we present a new type of atomic source: an ultra-narrow beam of metastable atoms produced by resonant metastability exchange inside a supersonic beam of rare gas atoms. We used the coherence properties of this beam to observe the diffraction of metastable helium, argon and neon atoms by a nano-transmission grating and by micro-reflection-gratings. Then, we evidenced transitions between Zeeman sublevels of neon metastable {sup 3}P{sub 2} state due to the quadrupolar part of Van der Waals potential. After we showed experimental proofs of the observation of this phenomenon, we calculated the transition probabilities in the Landau - Zener model. We discussed the interest of Van der Waals - Zeeman transitions for atom interferometry. Last, we described the Zeeman cooling of the supersonic metastable argon beam ({sup 3}P{sub 2}). We have succeeded in slowing down atoms to speeds below 100 m/s. We gave experimental details and showed the first time-of-flight measurements of slowed atoms.

  16. Size Determination of Argon Clusters from a Rayleigh Scattering Experiment

    Institute of Scientific and Technical Information of China (English)

    LEI An-Le; ZHAI Hua-Jin; LIU Bing-Chen; LI Zhong; NI Guo-Yuan; XU Zhi-Zhan

    2000-01-01

    Argon clusters are produced in the process of adiabatic expansion of a high backing pressure gas into vacuum through a nozzle. The cluster size is determined by a Rayleigh scattering measurement. The scattered signal measured is proportional to the 2.78th power of gas stagnation pressure. The average cluster sizes vary from 100 to more than 12000 atoms/cluster with the argon gas backing pressures ranging between 3 to 45 atm.

  17. Argon in action

    CERN Document Server

    Corinne Pralavorio

    2015-01-01

    Over the past few days, the SPS has been accelerating argon ions, which have started to be sent to the NA61/SHINE experiment. This operating mode, using a new type of ion, required a number of modifications to the accelerator.   Picture 1: a “super-cycle” of the SPS, featuring a proton cycle for the LHC, followed by an argon ion cycle for the North Area. Today, the accelerators are once again juggling particles and even performing completely new tricks. The SPS is supplying beams of argon ions for the first time, at energies never before achieved for this type of beam. They are destined for the NA61/SHINE experiment (see box) located in the North Area, which began receiving the beams on 11 February. Argon ions have a relatively large mass, as they consist of 40 nucleons, so they can be used in a similar way to lead ions. The main difficulty in accelerating them lies in the SPS, where the variation in acceleration frequency is limited. “The SPS was designed for a...

  18. Thermophysical properties of argon

    Energy Technology Data Exchange (ETDEWEB)

    Jaques, A.

    1988-02-01

    The entire report consists of tables of thermodynamic properties (including sound velocity, thermal conductivity and diffusivity, Prandtl number, density) of argon at 86 to 400/degree/K, in the form of isobars over 0.9 to 100 bars. (DLC)

  19. Optical and Electron Spin Resonance Studies of Destruction of Porous Structures Formed by Nitrogen-Rare Gas Nanoclusters in Bulk Superfluid Helium

    Science.gov (United States)

    McColgan, Patrick T.; Meraki, Adil; Boltnev, Roman E.; Lee, David M.; Khmelenko, Vladimir V.

    2016-11-01

    We studied optical and electron spin resonance spectra during destruction of porous structures formed by nitrogen-rare gas (RG) nanoclusters in bulk superfluid helium containing high concentrations of stabilized nitrogen atoms. Samples were created by injecting products of a radio frequency discharge of nitrogen-rare gas-helium gas mixtures into bulk superfluid helium. These samples have a high energy density allowing the study of energy release in chemical processes inside of nanocluster aggregates. The rare gases used in the studies were neon, argon, and krypton. We also studied the effects of changing the relative concentrations between nitrogen and rare gas on thermoluminescence spectra during destruction of the samples. At the beginning of the destructions, α -group of nitrogen atoms, Vegard-Kaplan bands of N_2 molecules, and β -group of O atoms were observed. The final destruction of the samples were characterized by a series bright flashes. Spectra obtained during these flashes contain M- and β -bands of NO molecules, the intensities of which depend on the concentration of molecular nitrogen in the gas mixture as well as the type of rare gas present in the gas mixture.

  20. Temporal evolution of electron beam generated Argon plasma in pasotron device

    Science.gov (United States)

    Khandelwal, Neha; Pal, U. N.; Prakash, Ram; Choyal, Y.

    2016-10-01

    The plasma- assisted slow wave oscillator (PASOTRON) is a high power microwave source in which the electron beam in the interaction region is confined by the background plasma. The plasma is generated by impact ionization of background gas with the electron beam. A model has been developed for temporal evolution of Argon plasma in pasotron device. In this model, we consider electron beam of energy E interacting with Argon gas. The resulting ionization creates quasi neutral argon plasma composed of argon Ar atoms, singly ionized ions Ar+1and electrons having energy from 0 to E. Electron impact excitation, ionization, radiative decay, radiative recombination and three body recombination processes are considered in this model. Population of ground and excited states of argon atom, ground state of argon ion as well as the population of electron energy groups is calculated by solving time dependent rate equations. Temporal evolution of electron beam generated plasma is given.

  1. Future liquid Argon detectors

    CERN Document Server

    Rubbia, A

    2013-01-01

    The Liquid Argon Time Projection Chamber offers an innovative technology for a new class of massive detectors for rare-event detection. It is a precise tracking device that allows three-dimensional spatial reconstruction with mm-scale precision of the morphology of ionizing tracks with the imaging quality of a "bubble chamber", provides $dE/dx$ information with high sampling rate, and acts as high-resolution calorimeter for contained events. First proposed in 1977 and after a long maturing process, its holds today the potentialities of opening new physics opportunities by providing excellent tracking and calorimetry performance at the relevant multi-kton mass scales, outperforming other techniques. In this paper, we review future liquid argon detectors presently being discussed by the neutrino physics community.

  2. Confined helium on Lagrange meshes

    CERN Document Server

    Baye, Daniel

    2015-01-01

    The Lagrange-mesh method has the simplicity of a calculation on a mesh and can have the accuracy of a variational method. It is applied to the study of a confined helium atom. Two types of confinement are considered. Soft confinements by potentials are studied in perimetric coordinates. Hard confinement in impenetrable spherical cavities is studied in a system of rescaled perimetric coordinates varying in [0,1] intervals. Energies and mean values of the distances between electrons and between an electron and the helium nucleus are calculated. A high accuracy of 11 to 15 significant figures is obtained with small computing times. Pressures acting on the confined atom are also computed. For sphere radii smaller than 1, their relative accuracies are better than $10^{-10}$. For larger radii up to 10, they progressively decrease to $10^{-3}$, still improving the best literature results.

  3. Particle detection by evaporation from superfluid helium

    Energy Technology Data Exchange (ETDEWEB)

    Bandler, S.R.; Lanou, R.E.; Maris, H.J.; More, T.; Porter, F.S.; Seidel, G.M.; Torii, R.H. (Department of Physics, Brown University, Providence, Rhode Island 02912 (United States))

    1992-04-20

    We report the first experiments in which 5-MeV alpha particles are detected via evaporation from a bath of superfluid helium. The {alpha} excites phonons and rotons in the liquid helium, and these excitations are sufficiently energetic to evaporate helium atoms when they reach the free surface of the liquid. The approximate overall efficiency of this process has been determined, and we compare this with expectations. We have also been able to detect evaporation induced by a flux of {gamma}'s from a {sup 137}Cs source.

  4. Rotational spectrum and dynamics of tetrahydrofuran-argon

    Energy Technology Data Exchange (ETDEWEB)

    Melandri, S.; Favero, P.G.; Caminati, W. [Dipartimento di Chimica ' G. Ciamician' dell' Universita, Via Selmi 2, I-40126 Bologna (Italy); Lopez, J.C.; Alonso, J.L. [Departamento de Quimica-Fisica, Facultad de Ciencias, Universidad de Valladolid, E-47005 Valladolid (Spain)

    1998-12-15

    The jet-cooled rotational spectrum of the tetrahydrofuran-argon molecular complex has been investigated by millimeter-wave absorption and Fourier transform microwave spectroscopies. The argon atom is located nearly over the oxygen atom, almost perpendicularly to the COC plane. Each rotational transition is split in two component lines due to the residual pseudorotational effects of the ring in the complex. The splitting between the two vibrational sublevels has been calculated to be 111.345(44) MHz. (Copyright (c) 1998 Elsevier Science B.V., Amsterdam. All rights reserved000.

  5. ATLAS Liquid Argon Calorimeter Module Zero

    CERN Multimedia

    1993-01-01

    This module was built and tested with beam to validate the ATLAS electromagnetic calorimeter design. One original design feature is the folding. 10 000 lead plates and electrodes are folded into an accordion shape and immersed in liquid argon. As they cross the folds, particles are slowed down by the lead. As they collide with the lead atoms, electrons and photons are ejected. There is a knock-on effect and as they continue on into the argon, a whole shower is produced. The electrodes collect up all the electrons and this signal gives a measurement of the energy of the initial particle. The M0 was fabricated by French institutes (LAL, LAPP, Saclay, Jussieu) in the years 1993-1994. It was tested in the H6/H8 beam lines in 1994, leading to the Technical Design Report in 1996.

  6. Explanation of the memory effect in argon

    Directory of Open Access Journals (Sweden)

    Marković Vidosav

    2005-01-01

    Full Text Available Memory effect - the long time variation of the electrical breakdown time delay on the relaxation time td (τ was observed in argon 24 hours after relaxation times and explained by the long-lived metastable states remaining from the preceding glow. However, the quenching processes reducing the effective lifetime of metastable states several orders of magnitude below that relevant for the time scale of observation were neglected. By applying approximate gas phase models it was found that the early afterglow kinetics up to hundreds of milliseconds is dominated by the decay of molecular argon ions Ar2+ and the approximate value of their ambipolar diffusion coefficient is determined. After that, nitrogen atoms present as impurities and recombined on the cathode surface and/or field emission determine the breakdown time delay down to the cosmic rays and natural radioactivity level.

  7. Annealing Behaviour of Helium Bubbles in Titanium Films by Thermal Desorption Spectroscopy and Positron Beam Analysis

    Institute of Scientific and Technical Information of China (English)

    LIU Chao-Zhuo; ZHOU Zhu-Ying; SHI Li-Qun; WANG Bao-Yi; HAO Xiao-Peng; ZHAO Guo-Qing

    2007-01-01

    @@ Helium-containing Ti films are prepared using magnetron sputtering in the helium-argon atmosphere. Isochronal annealing at different temperatures for an hour is employed to reveal the behaviour of helium bubble growth. Ion beam analysis is used to measure the retained helium content. Helium can release largely when annealing above 970 K. A thermal helium desorption spectroscopy system is constructed for assessment of the evolution of helium bubbles in the annealed samples by linear heating (0.4K/s) from room temperature to 1500K. Also, Doppler broadening measurements of positron annihilation radiation spectrum are performed by using changeable energy positron beam. Bubble coarsening evolves gradually below 680K, migration and coalescence of small bubbles dominates in the range of 680-970K, and the Ostwald ripening mechanism enlarges the bubbles with a massive release above 970K.

  8. Helium Tagging Infrared Photodissociation Spectroscopy of Reactive Ions.

    Science.gov (United States)

    Roithová, Jana; Gray, Andrew; Andris, Erik; Jašík, Juraj; Gerlich, Dieter

    2016-02-16

    The interrogation of reaction intermediates is key for understanding chemical reactions; however their direct observation and study remains a considerable challenge. Mass spectrometry is one of the most sensitive analytical techniques, and its use to study reaction mixtures is now an established practice. However, the information that can be obtained is limited to elemental analysis and possibly to fragmentation behavior, which is often challenging to analyze. In order to extend the available experimental information, different types of spectroscopy in the infrared and visible region have been combined with mass spectrometry. Spectroscopy of mass selected ions usually utilizes the powerful sensitivity of mass spectrometers, and the absorption of photons is not detected as such but rather translated to mass changes. One approach to accomplish such spectroscopy involves loosely binding a tag to an ion that will be removed by absorption of one photon. We have constructed an ion trapping instrument capable of reaching temperatures that are sufficiently low to enable tagging by helium atoms in situ, thus permitting infrared photodissociation spectroscopy (IRPD) to be carried out. While tagging by larger rare gas atoms, such as neon or argon is also possible, these may cause significant structural changes to small and reactive species, making the use of helium highly beneficial. We discuss the "innocence" of helium as a tag in ion spectroscopy using several case studies. It is shown that helium tagging is effectively innocent when used with benzene dications, not interfering with their structure or IRPD spectrum. We have also provided a case study where we can see that despite its minimal size there are systems where He has a huge effect. A strong influence of the He tagging was shown in the IRPD spectra of HCCl(2+) where large spectral shifts were observed. While the presented systems are rather small, they involve the formation of mixtures of isomers. We have therefore

  9. Communication: Dopant-induced solvation of alkalis in liquid helium nanodroplets

    Science.gov (United States)

    Renzler, Michael; Daxner, Matthias; Kranabetter, Lorenz; Kaiser, Alexander; Hauser, Andreas W.; Ernst, Wolfgang E.; Lindinger, Albrecht; Zillich, Robert; Scheier, Paul; Ellis, Andrew M.

    2016-11-01

    Alkali metal atoms and small alkali clusters are classic heliophobes and when in contact with liquid helium they reside in a dimple on the surface. Here we show that alkalis can be induced to submerge into liquid helium when a highly polarizable co-solute, C60, is added to a helium nanodroplet. Evidence is presented that shows that all sodium clusters, and probably single Na atoms, enter the helium droplet in the presence of C60. Even clusters of cesium, an extreme heliophobe, dissolve in liquid helium when C60 is added. The sole exception is atomic Cs, which remains at the surface.

  10. The muonic helium lamb shift experiment

    Energy Technology Data Exchange (ETDEWEB)

    Goetzfried, Johannes; Krauth, Julian [Max-Planck-Institute of Quantum Optics, Garching (Germany); Collaboration: CREMA collaboration

    2014-07-01

    Because of its high sensitivity on finite size effects of the nucleus, the measurement of the Lamb shift in exotic atoms has been on the wish-list of atomic and nuclear physics for a long time. Our previous experiment allowed to determine the proton radius with an order of magnitude higher precision compared to spectroscopic measurements of ordinary hydrogen. The successor experiment in muonic helium is currently performed at the Paul-Scherrer-Institute in Switzerland. Using a low energy muon beam line muons are stopped within low pressure helium gas, where exotic atoms are created. Here we measure the 2S-2P transition frequency of muonic helium illuminated by a pulsed TiSa-laser system pumped with a newly developed Yb-YAG thin disk laser. This measurement will ultimately improve the values of the charge radii of {sup 3}He{sup +} and {sup 4}He{sup +} by an order of magnitude.

  11. Atomistic simulation of helium bubble nucleation in palladium

    Energy Technology Data Exchange (ETDEWEB)

    Wang Liang [Department of Applied Physics, Hunan University, Changsha 410082 (China); Hu, Wangyu [Department of Applied Physics, Hunan University, Changsha 410082 (China)], E-mail: wangyuhu2001cn@yahoo.com.cn; Xiao Shifang [Department of Applied Physics, Hunan University, Changsha 410082 (China)], E-mail: sfxiao@yahoo.com.cn; Yang Jianyu [Department of Maths and Physics, Hunan Institute of Engineering, Xiangtan 411104 (China); Deng Huiqiu [Department of Applied Physics, Hunan University, Changsha 410082 (China)

    2009-09-15

    A palladium crystal has been constructed with 11808 atoms. 55 helium atoms occupied the octahedral position of palladium crystal are introduced and retained in a spherical region. Molecular dynamic simulations are performed in a constant temperature and constant volume ensemble (NVT) with temperature controlled by Nose-Hoover thermostat. The interactions between palladium atoms are described with modified analytic embedded atom method (MAEAM), the interactions between palladium atom and helium atom are in the form of Morse potential, and the interactions between helium atoms are in the form of L-J potential function. With the analysis of the radial distribution function (RDF) and microstructure, it reveals that some of helium atoms form a series of clusters with different size, and the nucleation core is random at low temperature, and which is the embryo of helium bubble. Increasing temperature can accelerate the process of bubble nucleation, and the clusters will aggregate and coalesce into a bigger one in which there are no palladium atoms, and it is considered as a helium bubble.

  12. Influence of helium atoms on the shear behavior of the fiber/matrix interphase of SiC/SiC composite

    Science.gov (United States)

    Jin, Enze; Du, Shiyu; Li, Mian; Liu, Chen; He, Shihong; He, Jian; He, Heming

    2016-10-01

    Silicon carbide has many attractive properties and the SiC/SiC composite has been considered as a promising candidate for nuclear structural materials. Up to now, a computational investigation on the properties of SiC/SiC composite varying in the presence of nuclear fission products is still missing. In this work, the influence of He atoms on the shear behavior of the SiC/SiC interphase is investigated via Molecular Dynamics simulation following our recent paper. Calculations are carried out on three dimensional models of graphite-like PyC/SiC interphase and amorphous PyC/SiC interphase with He atoms in different regions (the SiC region, the interface region and the PyC region). In the graphite-like PyC/SiC interphase, He atoms in the SiC region have little influence on the shear strength of the material, while both the shear strength and friction strength may be enhanced when they are in the PyC region. Low concentration of He atoms in the interface region of the graphite-like PyC/SiC interphase increases the shear strength, while there is a reduction of shear strength when the He concentration is high due to the switch of sliding plane. In the amorphous PyC/SiC interphase, He atoms can cause the reduction of the shear strength regardless of the regions that He atoms are located. The presence of He atoms may significantly alter the structure of SiC/SiC in the interface region. The influence of He atoms in the interface region is the most significant, leading to evident shear strength reduction of the amorphous PyC/SiC interphase with increasing He concentration. The behaviors of the interphases at different temperatures are studied as well. The dependence of the shear strengths of the two types of interphases on temperatures is studied as well. For the graphite-like PyC/SiC interphase, it is found strongly related to the regions He atoms are located. Combining these results with our previous study on pure SiC/SiC system, we expect this work may provide new insight

  13. Influence of Additive Gas on Electrical and Optical Characteristics of Non-equilibrium Atmospheric Pressure Argon Plasma Jet%Influence of Additive Gas on Electrical and Optical Characteristics of Non-equilibrium Atmospheric Pressure Argon Plasma Jet

    Institute of Scientific and Technical Information of China (English)

    费小猛; Shin-ichi KURODA; Yuki KONDO; Tamio MORI; Katsuhiko HOSOI

    2011-01-01

    Electrical and optical properties of an argon plasma jet were characterized. In particular, effects of an additive gas, namely nitrogen or oxygen, on these properties were studied in detail. The plasma jet was found to be of a glow-like discharge, which scarcely changed upon the injection of an additive gas, either directly or through a glass capillary. Optical emission spectroscopy characterization revealed that excited argon atoms were the predominant active species in this plasma jet. Metastable argon atoms were highly quenched, and N2(C3yIu) became the main energy carrier following nitrogen injection. When oxygen was added to the afterglow zone through a glass capillary, no significant quenching effect was observed and the number of oxygen atoms decreased with the increase in oxygen concentration. Finally, to demonstrate an application of this plasma jet, a high-density polyethylene surface was treated with argon, argon/nitrogen, and argon/oxygen plasmas.

  14. Fano Resonances observed in Helium Nanodroplets

    CERN Document Server

    LaForge, A C; Jabbari, G; Gokhberg, K; Kryzhevoi, N V; Krishnan, S R; Hess, M; O'Kee?e, P; Ciavardini, A; Prince, K C; Richter, R; Moshammer, R; Cederbaum, L S; Pfeifer, T; Stienkemeier, F; Mudrich, M

    2015-01-01

    Doubly-excited Rydberg states of helium (He) nanodroplets have been studied using synchrotron radiation. We observed Fano resonances related to the atomic N = 2,0 series as a function of droplet size. Although similar qualitatively to their atomic counterparts, the resonance lines are broader and exhibit a shift in energy which increases for the higher excited states. Furthermore, additional resonances are observed which are not seen in atomic systems. We discuss these features in terms of delocalized atomic states perturbed by the surrounding He atoms and compare to singly excited droplets.

  15. Particle detection using superfluid helium

    Energy Technology Data Exchange (ETDEWEB)

    Bandler, S.R.; Lanou, R.E.; Maris, H.J.; More, T.; Porter, F.S.; Seidel, G.M.; Torii, R.

    1991-01-01

    We have observed 5 MeV {alpha} particles stopped in volumes-up to two liters of liquid helium at 70 mK. A fraction of the kinetic energy of an {alpha} particle is converted to elementary excitations (rotons and phonons), which progagate ballistically in isotopically pure {sup 4}He below 0.1 K. Most of these excitations have sufficient energy to evaporate helium atoms on hitting a free surface. The evaporated helium atoms can be detected calorimetrically when adsorbed on a thin silicon wafer ({approximately}1.7 g, 35 cm{sup 2}) suspended above the liquid. Temperature changes of the silicon are measured with a NTD germanium bolometer. For the geometry studied the observed temperature change of the silicon resulting from an {alpha} event in the liquid is approximately 5% of the temperature rise from an {alpha} hitting the silicon directly. The implications of these measurements will be discussed as they relate to the possible construction of a large scale detector of solar neutrinos.

  16. Particle detection using superfluid helium

    Energy Technology Data Exchange (ETDEWEB)

    Bandler, S.R.; Lanou, R.E.; Maris, H.J.; More, T.; Porter, F.S.; Seidel, G.M.; Torii, R.

    1991-12-31

    We have observed 5 MeV {alpha} particles stopped in volumes-up to two liters of liquid helium at 70 mK. A fraction of the kinetic energy of an {alpha} particle is converted to elementary excitations (rotons and phonons), which progagate ballistically in isotopically pure {sup 4}He below 0.1 K. Most of these excitations have sufficient energy to evaporate helium atoms on hitting a free surface. The evaporated helium atoms can be detected calorimetrically when adsorbed on a thin silicon wafer ({approximately}1.7 g, 35 cm{sup 2}) suspended above the liquid. Temperature changes of the silicon are measured with a NTD germanium bolometer. For the geometry studied the observed temperature change of the silicon resulting from an {alpha} event in the liquid is approximately 5% of the temperature rise from an {alpha} hitting the silicon directly. The implications of these measurements will be discussed as they relate to the possible construction of a large scale detector of solar neutrinos.

  17. Création d'atomes d'argon excités dans des états de Rydberg en vue de l'étude de l'autodétachement électronique d'ions moléculaires SF6 -6 dans un piège quadrupolaire radiofréquence

    OpenAIRE

    Brincourt, G.; Vedel, M.; Zerega, Y.; André, J; Vedel, F.

    1982-01-01

    Nous décrivons dans ce travail les conditions expérimentales d'obtention d'atomes d'argon excités dans des états de Rydberg par bombardement électronique. Nous précisons certaines de leurs propriétés qu'il est nécessaire de connaître dans la perspective de l'étude de l'auto-détachement électronique d'ions moléculaires SF6-dans un piège quadrupolaire radiofréquence. Ces ions sont créés par interaction, à énergie quasi-nulle, de molécules SF6 avec des atomes excités dans des états de Rydberg. D...

  18. Helium on Venus - Implications for uranium and thorium

    Science.gov (United States)

    Prather, M. J.; Mcelroy, M. B.

    1983-01-01

    Helium is removed at an average rate of 10 to the 6th atoms per square centimeter per second from Venus's atmosphere by the solar wind following ionization above the plasmapause. The surface source of helium-4 on Venus is similar to that on earth, suggesting comparable abundances of crustal uranium and thorium.

  19. Experimental studies of antiprotonic helium

    CERN Document Server

    Widmann, E

    1998-01-01

    This talk describes the experimental studies of metastable antiprotonic helium "atomcules" pHe/sup +/ (a neutral exotic atom consisting of a helium nucleus, an antiproton and an electron) performed at CERN-LEAR, and future plans for experiments at the forthcoming Antiproton Decelerator (AD) at CERN. Laser spectroscopy experiments are reviewed which led to the observation of a total of 13 resonant transitions of the antiproton in both p/sup 4/He/sup +/ and p/sup 3/He/sup +/, and revealed a hyperfine splitting in one transition. A level of precision has been reached where the most accurate 3-body calculations need to include QED effects like the Lamb-shift to come close to the experimental results. (52 refs).

  20. Rapidly pulsed helium droplet source

    Energy Technology Data Exchange (ETDEWEB)

    Pentlehner, Dominik; Riechers, Ricarda; Dick, Bernhard; Slenczka, Alkwin [Institute for Physical and Theoretical Chemistry, University of Regensburg, 93053 Regensburg (Germany); Even, Uzi; Lavie, Nachum; Brown, Raviv; Luria, Kfir [Sackler Faculty of Exact Sciences, School of Chemistry, Tel Aviv University, Ramat Aviv, 69978 Tel Aviv (Israel)

    2009-04-15

    A pulsed valve connected to a closed-cycle cryostat was optimized for producing helium droplets. The pulsed droplet beam appeared with a bimodal size distribution. The leading part of the pulse consists of droplets suitable for doping with molecules. The average size of this part can be varied between 10{sup 4} and 10{sup 6} helium atoms, and the width of the distribution is smaller as compared to a continuous-flow droplet source. The system has been tested in a single pulse mode and at repetition rates of up to 500 Hz with almost constant intensity. The droplet density was found to be increased by more than an order of magnitude as compared to a continuous-flow droplet source.

  1. Spectroscopic studies of OCS-doped 4He clusters with 9-72 helium atoms: observation of broad oscillations in the rotational moment of inertia.

    Science.gov (United States)

    McKellar, A R W; Xu, Yunjie; Jäger, Wolfgang

    2007-08-09

    High-resolution spectra of HeN-OCS clusters with N up to 39 in the microwave region and up to 72 in the infrared region were observed with apparatus-limited line widths of about 15 kHz and 0.001 cm(-1), respectively. The cold (approximately 0.2 K) clusters were produced in pulsed supersonic jet expansions of very dilute OCS + He mixtures and probed using a microwave Fourier transform spectrometer or a tunable infrared diode laser spectrometer. Consistent analyses of the microwave and infrared data yield band origins for the carbonyl stretching vibration, together with rotational parameters for the ground and excited vibrational states. The rotational constant, B, passes through a minimum at N = 9 and then rises as the He atoms uncouple from the OCS rotational motion as a result of superfluid effects. There are broad unexpected oscillations in B, with maxima at N = 24 and 47 and minima at N = 36 and 62. The change in B upon vibrational excitation, which is negative for the OCS molecule, converges to positive values for N > 15. These results help to bridge the gap between individual molecules and bulk matter with atom-by-atom resolution over a significant range of cluster sizes.

  2. Exotic helium molecules; Molecules exotiques d'helium

    Energy Technology Data Exchange (ETDEWEB)

    Portier, M

    2007-12-15

    We study the photo-association of an ultracold cloud of magnetically trapped helium atoms: pairs of colliding atoms interact with one or two laser fields to produce a purely long range {sup 4}He{sub 2}(2{sup 3}S{sub 1}-2{sup 3}P{sub 0}) molecule, or a {sup 4}He{sub 2}(2{sup 3}S{sub 1}-2{sup 3}S{sub 1}) long range molecule. Light shifts in one photon photo-association spectra are measured and studied as a function of the laser polarization and intensity, and the vibrational state of the excited molecule. They result from the light-induced coupling between the excited molecule, and bound and scattering states of the interaction between two metastable atoms. Their analysis leads to the determination of the scattering length a = (7.2 {+-} 0.6) ruling collisions between spin polarized atoms. The two photon photo-association spectra show evidence of the production of polarized, long-range {sup 4}He{sub 2}(2{sup 3}S{sub 1}-2{sup 3}S{sub 1}) molecules. They are said to be exotic as they are made of two metastable atoms, each one carrying a enough energy to ionize the other. The corresponding lineshapes are calculated and decomposed in sums and products of Breit-Wigner and Fano profiles associated to one and two photon processes. The experimental spectra are fit, and an intrinsic lifetime {tau} = (1.4 {+-} 0.3) {mu}s is deduced. It is checked whether this lifetime could be limited by spin-dipole induced Penning autoionization. This interpretation requires that there is a quasi-bound state close to the dissociation threshold in the singlet interaction potential between metastable helium atoms for the theory to match the experiment. (author)

  3. Helium vs. Proton Induced Displacement Damage in Electronic Materials

    Science.gov (United States)

    Ringo, Sawnese; Barghouty, A. F.

    2010-01-01

    In this project, the specific effects of displacement damage due to the passage of protons and helium nuclei on some typical electronic materials will be evaluated and contrasted. As the electronic material absorbs the energetic proton and helium momentum, degradation of performance occurs, eventually leading to overall failure. Helium nuclei traveling at the same speed as protons are expected to impart more to the material displacement damage; due to the larger mass, and thus momentum, of helium nuclei compared to protons. Damage due to displacement of atoms in their crystalline structure can change the physical properties and hence performance of the electronic materials.

  4. Catching proteins in liquid helium droplets

    CERN Document Server

    Kupser, Peter; Meijer, Gerard; von Helden, Gert

    2010-01-01

    An experimental approach is presented that allows for the incorporation of large mass/charge selected ions in liquid helium droplets. It is demonstrated that droplets can be efficiently doped with a mass/charge selected amino acid as well as with the much bigger m$\\approx$12 000 amu protein Cytochrome C in selected charge states. The sizes of the ion-doped droplets are determined via electrostatic deflection. Under the experimental conditions employed, the observed droplet sizes are very large and range, dependent on the incorporated ion, from 10$^{10}$ helium atoms for protonated Phenylalanine to 10$^{12}$ helium atoms for Cytochrome C. As a possible explanation, a simple model based on the size- and internal energy-dependence of the pickup efficiency is given.

  5. Cross section measurements of the processes occurring in the fragmentation of H{sub n}{sup +} (3 {<=} n {<=} 35) hydrogen clusters induced by high speed (60 keV/u) collisions on helium atoms; Mesure des sections efficaces des differents processus intervenant dans la fragmentation d`agregats d`hydrogene H{sub n}{sup +} (3 {<=} n {<=} 35) induite par collision a haute vitesse (60 keV/u) sur un atome d`helium

    Energy Technology Data Exchange (ETDEWEB)

    Louc, Sandrine [Inst. de Physique Nucleaire, Lyon-1 Univ., 69 - Villeurbanne (France)

    1997-09-15

    Different processes involved in the fragmentation of ionised hydrogen clusters H{sub 3} + (H{sub 2}){sub (n-3)/2} (n = 5-35) have been studied in the same experiment: the fragmentation of the cluster is induced by the collision with an helium atom at high velocity ({approx_equal} c/100). The collision is realised in reversed kinematic - clusters are accelerated - which allows the detection of neutral and charged fragments. The different channels of fragmentation are identified by using coincidence techniques. For all the cluster sizes studied the capture cross sections of one electron of the target by the cluster is equal to the capture cross section of the H{sub 3}{sup +} ion. In the same way, the dissociation cross section of the H{sub 3}{sup +} core of the cluster does not depend on cluster size. These fragmentation processes are due to the interaction of H{sub 3}{sup +} core of the cluster and the helium atom without ionization of another component of the cluster. On the contrary, the cross sections of loss of one, two and three molecules by the cluster and the dissociation cross section of the cluster in all its molecular components depends strongly on the cluster size. This dependence is different from the one measured for the metastable decay of the cluster. Thus, the process of loss of molecules induced by a collision should correspond to a different dissociation mechanism. In regard of the singularities observed for the size dependence, the H{sub 9}{sup +}, H{sub 15}{sup +}, H{sub 19}{sup +} and H{sub 29}{sup +} clusters could be the `core` of the biggest clusters. These observation are in agreement with the size effects of smaller magnitude observed for the dissociation cross section (all the processes). The values of the cross section for the process of at least one ionization of the cluster indicate that about 80% of the fragmentation events result from this process. (author) 114 refs., 74 figs., 9 tabs.

  6. Wetting and evaporation of argon nanodroplets on smooth and rough substrates: Molecular dynamics simulations

    Science.gov (United States)

    Li, Qun; Wang, Baohe; Chen, Yonggang; Zhao, Zongchang

    2016-10-01

    Wetting and evaporation behaviors of argon nanodroplets on smooth and rough substrates are studied using molecular dynamics simulations. Effects of interaction energy between solid and argon atoms on wetting and evaporation and differences between nanodroplets on smooth and rough substrates have been investigated. The results show that for both smooth and rough substrates, as the interaction energy between solid and argon atoms increases, the contact angle and total evaporation increase. For rough substrates, the variations of contact angle and contact radius during evaporation progress are much more complex and the total evaporation is much larger than that of smooth substrates.

  7. Atomic physics

    Energy Technology Data Exchange (ETDEWEB)

    Livingston, A.E.; Kukla, K.; Cheng, S. [Univ. of Toledo, OH (United States)] [and others

    1995-08-01

    In a collaboration with the Atomic Physics group at Argonne and the University of Toledo, the Atomic Physics group at the University of Notre Dame is measuring the fine structure transition energies in highly-charged lithium-like and helium-like ions using beam-foil spectroscopy. Precise measurements of 2s-2p transition energies in simple (few-electron) atomic systems provide stringent tests of several classes of current atomic- structure calculations. Analyses of measurements in helium-like Ar{sup 16+} have been completed, and the results submitted for publication. A current goal is to measure the 1s2s{sup 3}S{sub 1} - 1s2p{sup 3}P{sub 0} transition wavelength in helium-like Ni{sup 26+}. Measurements of the 1s2s{sup 2}S{sub 1/2} - 1s2p{sup 2}P{sub 1/2,3/2} transition wavelengths in lithium-like Kr{sup 33+} is planned. Wavelength and lifetime measurements in copper-like U{sup 63+} are also expected to be initiated. The group is also participating in measurements of forbidden transitions in helium-like ions. A measurement of the lifetime of the 1s2s{sup 3}S{sub 1} state in Kr{sup 34+} was published recently. In a collaboration including P. Mokler of GSI, Darmstadt, measurements have been made of the spectral distribution of the 2E1 decay continuum in helium-like Kr{sup 34+}. Initial results have been reported and further measurements are planned.

  8. Depleted argon from underground sources

    Energy Technology Data Exchange (ETDEWEB)

    Back, H.O.; /Princeton U.; Alton, A.; /Augustana U. Coll.; Calaprice, F.; Galbiati, C.; Goretti, A.; /Princeton U.; Kendziora, C.; /Fermilab; Loer, B.; /Princeton U.; Montanari, D.; /Fermilab; Mosteiro, P.; /Princeton U.; Pordes, S.; /Fermilab

    2011-09-01

    Argon is a powerful scintillator and an excellent medium for detection of ionization. Its high discrimination power against minimum ionization tracks, in favor of selection of nuclear recoils, makes it an attractive medium for direct detection of WIMP dark matter. However, cosmogenic {sup 39}Ar contamination in atmospheric argon limits the size of liquid argon dark matter detectors due to pile-up. The cosmic ray shielding by the earth means that Argon from deep underground is depleted in {sup 39}Ar. In Cortez Colorado a CO{sub 2} well has been discovered to contain approximately 500ppm of argon as a contamination in the CO{sub 2}. In order to produce argon for dark matter detectors we first concentrate the argon locally to 3-5% in an Ar, N{sub 2}, and He mixture, from the CO{sub 2} through chromatographic gas separation. The N{sub 2} and He will be removed by continuous cryogenic distillation in the Cryogenic Distillation Column recently built at Fermilab. In this talk we will discuss the entire extraction and purification process; with emphasis on the recent commissioning and initial performance of the cryogenic distillation column purification.

  9. Observation of double resonant laser induced transitions in the $v = n - l - 1 = 2$ metastable cascade of antiprotonic helium-4 atoms

    CERN Document Server

    Hayano, R S; Tamura, H; Torii, H A; Hori, Masaki; Maas, F E; Morita, N; Kumakura, M; Sugai, I; Hartmann, F J; Daniel, H; Von Egidy, T; Ketzer, B; Pohl, R; Horváth, D; Eades, John; Widmann, E; Yamazaki, T

    1997-01-01

    A new laser-induced resonant transition in the $v=n-l-1=2$ metastable cascade of antiprotonic $^4$He atoms has been found by using a double resonance technique. This was done by setting the first laser to the already known 470.724 nm resonance ($(n,l)=(37,34)\\rightarrow (36,33)$), while the $(38,35)\\rightarrow (37,34)$ transition was searched for with the second laser. The resonant transition was found at wavelength of 529.622$\\pm$0.003 nm, showing excellent agreement with a recent prediction of Korobov.

  10. Investigation of Non-Equilibrium Argon and Hydrogen Plasmas.

    Science.gov (United States)

    Braun, Christopher Gifford

    1987-09-01

    Theoretical and experimental investigations are made into non-equilibrium argon and hydrogen partially -ionized plasmas characteristic of glow discharge devices such as thyratrons and discharge tubes. For an argon plasma, the development and use of a collisional-radiative, steady -state, three-energy-level model is presented and experimental measurements on pulsed argon plasmas are briefly mentioned. Two different theoretical argon plasma models are discussed; the first is numerically solved using a non-Maxwellian electron distribution function, while the second is solved analytically, including atom-atom inelastic collisions, assuming Maxwellian electron and atom distribution functions. For a hydrogen plasma, experimental measurements using fluorescence and laser-induced fluorescence have been made in a modified hydrogen thyratron over a wide current density range (from 100 to 8,000 A/cm('2)) for the atomic hydrogen population densities n = 2,3,4. A pronounced rise in the atomic hydrogen excited state populations is observed after the end of the current pulse. A new method to measure the time-resolved electron density has been developed and results are presented. A time-dependent model for atomic hydrogen plasmas typical of a thyratron has been constructed, and preliminary results are shown. This model includes ten atomic energy levels (n = 1 to n = 9 and the continuum), takes into account energy balance with an externally supplied current density and assumes a Maxwellian electron distribution function. Implications of these measurements and theoretical analysis upon the operation of thyratrons are discussed. (Copies available exclusively from Micrographics Department, Doheny Library, University of Southern California, Los Angeles, CA 90089 -0182.).

  11. Thermalization of magnetically trapped metastable helium

    CERN Document Server

    Browaeys, A; Sirjean, O; Poupard, J; Nowak, S; Boiron, D; Westbrook, C I; Aspect, Alain

    2001-01-01

    We have observed thermalization by elastic collisions of magnetically trapped metastable helium atoms. Our method directly samples the reconstruction of a thermal energy distribution after the application of an RF knife. The relaxation time of our sample towards equilibrium gives an elastic collision rate constant close to the unitarity limit.

  12. Interaction of Helium Rydberg State Molecules with Dense Helium.

    Science.gov (United States)

    Bonifaci, Nelly; Li, Zhiling; Eloranta, Jussi; Fiedler, Steven L

    2016-11-17

    The interaction potentials of the He2(*) excimer, in the a(3)Σu, b(3)Πg, c(3)Σg, and d(3)Σu electronic states with a ground state helium atom are presented. The symmetry of the interaction potentials closely follows the excimer Rydberg electron density with pronounced short-range minima appearing along the nodal planes of the Rydberg orbital. In such cases, a combination of the electrostatic short-range attraction combined with Pauli repulsion leads to the appearance of unusual long-range maxima in the potentials. Bosonic density functional calculations show that the (3)d state excimer resides in a localized solvation bubble in dense helium at 4.5 K, with radii varying from 12.7 Å at 0.1 MPa to 10.8 Å at 2.4 MPa. The calculated (3)d → (3)b pressure-induced fluorescence band shifts are in good agreement with experimental results determined by application of corona discharge. The magnitude of the spectral shifts indicate that the observed He2(*) molecules emit from dense helium whereas the corresponding fluorescence signal from the discharge zone appears quenched. This implies that fluorescence spectroscopy involving this electronic transition can only be used to probe the state of the surrounding medium rather than the discharge zone itself.

  13. Full Scale Thermo-hydraulic Simulation of a Helium-Helium Printed Circuit Heat Exchanger

    Energy Technology Data Exchange (ETDEWEB)

    Lee, Injun; Hong, Sungyull; Bai, Cheolho; Shim, Jaesool [Yeungnam Univ., Gyeongsan (Korea, Republic of); Kim, Chansoo; Hong, Sungdeok; Kim, Minhwan [Korea Atomic Energy Research Institute, Daejeon (Korea, Republic of)

    2014-05-15

    In this paper, the thermo-hydraulic full scale simulation is performed to study the temperature distributions, thermal stress, pressure drop and outlet temperature in a Helium-Helium printed circuit heat exchanger (PCHE) in a VHTR simulate helium loop. The entire PCHE is composed of 40 stacks of rectangular shaped micro-channels for helium gas [type A] (inlet temperature, 400 .deg. C) and 40 stacks of semi-ellipse shaped micro-channels for helium [type B] (inlet temperature, 300 .deg. C). The experimental result is compared to that of computer simulation, COMSOL multi-physics software. The Helium-Helium PCHE is considered a prototype of the newly developed PCHE by Korea Atomic Energy Research Institute (KAERI). The full scale thermo-hydraulic simulation was successfully performed to obtain temperature distribution, pressure drop and thermal stress in 40 sets of flow channel stacks in a helium-helium printed circuit heat exchanger in a VHTR simulate helium loop. We obtained a quite similar temperature distribution with the 3D measured infrared temperature distribution. To our knowledge, this is the first full scale numerical study on the PCHE, which considers all microchannels, that the convection effect on the outside surfaces of the PCHE is applied. The very high-temperature reactor (VHTR) or high-temperature gas-cooled reactor(HTGR) is a fourth-generation nuclear power reactor that uses the ceramic coated fuel, TRISO, in which the fission gas does not leak even at temperatures higher than 1600 .deg. C. The VHTR necessarily requires an intermediate loop composed of a hot gas duct (HGD), an intermediate heat exchanger (IHX) and a process heat exchanger (PHE). The IHX is one of the important components of VHTR system because the IHX transfers the 950 .deg. C of high temperature massive heat to a hydrogen production plant or power conversion unit at high system pressure.

  14. Solvation of Na+, K+, and Their Dimers in Helium

    OpenAIRE

    An der Lan, Lukas; Bartl, Peter; Leidlmair, Christian; Jochum, Roland; Denifl, Stephan; Echt, Olof; Scheier, Paul

    2012-01-01

    Helium atoms bind strongly to alkali cations which, when embedded in liquid helium, form so-called snowballs. Calculations suggest that helium atoms in the first solvation layer of these snowballs form rigid structures and that their number (n) is well defined, especially for the lighter alkalis. However, experiments have so far failed to accurately determine values of n. We present high-resolution mass spectra of Na+He n , K+He n , Na2 +He n and K2 +He n , formed by electron ionization of do...

  15. The Liquid Argon Purity Demonstrator

    CERN Document Server

    Adamowski, M; Dvorak, E; Hahn, A; Jaskierny, W; Johnson, C; Jostlein, H; Kendziora, C; Lockwitz, S; Pahlka, B; Plunkett, R; Pordes, S; Rebel, B; Schmitt, R; Stancari, M; Tope, T; Voirin, E; Yang, T

    2014-01-01

    The Liquid Argon Purity Demonstrator was an R&D test stand designed to determine if electron drift lifetimes adequate for large neutrino detectors could be achieved without first evacuating the cryostat. We describe here the cryogenic system, its operations, and the apparatus used to determine the contaminant levels in the argon and to measure the electron drift lifetime. The liquid purity obtained by this system was facilitated by a gaseous argon purge. Additionally, gaseous impurities from the ullage were prevented from entering the liquid at the gas-liquid interface by condensing the gas and filtering the resulting liquid before returning to the cryostat. The measured electron drift lifetime in this test was greater than 6 ms, sustained over several periods of many weeks. Measurements of the temperature profile in the argon, to assess convective flow and boiling, were also made and are compared to simulation.

  16. The Liquid Argon Purity Demonstrator

    Energy Technology Data Exchange (ETDEWEB)

    Adamowski, M.; Carls, B.; Dvorak, E.; Hahn, A.; Jaskierny, W.; Johnson, C.; Jostlein, H.; Kendziora, C.; Lockwitz, S.; Pahlka, B.; Plunkett, R.; Pordes, S.; Rebel, B.; Schmitt, R.; Stancari, M.; Tope, T.; Voirin, E.; Yang, T.

    2014-07-01

    The Liquid Argon Purity Demonstrator was an R&D test stand designed to determine if electron drift lifetimes adequate for large neutrino detectors could be achieved without first evacuating the cryostat. We describe here the cryogenic system, its operations, and the apparatus used to determine the contaminant levels in the argon and to measure the electron drift lifetime. The liquid purity obtained by this system was facilitated by a gaseous argon purge. Additionally, gaseous impurities from the ullage were prevented from entering the liquid at the gas-liquid interface by condensing the gas and filtering the resulting liquid before returning to the cryostat. The measured electron drift lifetime in this test was greater than 6 ms, sustained over several periods of many weeks. Measurements of the temperature profile in the argon, to assess convective flow and boiling, were also made and are compared to simulation.

  17. Metal clusters on supported argon layers; Metallcluster auf dielektrischen Substraten

    Energy Technology Data Exchange (ETDEWEB)

    Faber, Bernhard

    2011-10-21

    The deposition of small sodium clusters on supported Ar(001)-surfaces is simulated. Theoretical description is achieved by a hierarchical model consisting of time-dependent DFT and molecular dynamics. The valence electrons of the sodium atoms are considered by Kohn-Sham-Scheme with self interaction correction. The interaction of argon atoms and sodium ions is described by atom-atom potentials whereas the coupling to the QM electrons is done by local pseudo-potentials. A decisive part of the model is the dynamical polarizability of the rare-gas atoms. The optional metal support is considered by the method of image charges. The influence of the forces caused by image charges and the influence of the number of argon monolayers on structure, optical response and deposition dynamics of Na{sub 6} and Na{sub 8} is investigated. There is very little influence on cluster structure and only a small shift of the cluster perpendicular to the surface. Concerning optical response the position of the Mie plasmon peak stays robust whereas the details of spectral fragmentation react very sensitively to changes. The forces caused by image charges of the metal support play only a little role with the dynamics of deposition while the thickness of the argon surface strongly influences the dissipation. (orig.)

  18. Thermal Annealing Behavior of Helium in Ti Films Deposited by Magnetron Sputtering

    Institute of Scientific and Technical Information of China (English)

    ZHANG Lei; HE Zhi-Jiang; LIU Chao-Zhuo; WANG Xu-Fei; SHI Li-Qun

    2012-01-01

    Helium contents of up to 30at.% are prepared in sputter-deposited Ti Silms. Isochronal annealing behaviors of helium including the depth profiles and the evolution of helium bubbles in the fi1ms at different temperatures are examined by ion beam analysis including Rutherford backscattering spectrometry (RBS) and elastic recoil detection analysis (ERDA), as well as thermal helium desorption spectroscopy (THDS). It is found that the energy spreading induced by structural inhomogeneities in the spectra of RBS and ERDA as well as the increment in the width of spectra occurs, which corresponds to the change of stopping cross-section of helium atoms in the Ti 61m due to the change of physical-state of helium in the evolution of helium bubble. The ion beam analysis on the helium evolution is consistent with the THDS measurement. Ion beam technique opens interesting possibilities in the characterizing on the growth of helium bubbles.%Helium contents of up to 30at.% are prepared in sputter-deposited Ti films.Isochronal annealing behaviors of helium including the depth profiles and the evolution of helium bubbles in the films at different temperatures are examined by ion beam analysis including Rutherford backscattering spectrometry (RBS) and elastic recoil detection analysis (ERDA),as well as thermal helium desorption spectroscopy (THDS).It is found that the energy spreading induced by structural inhomogeneities in the spectra of RBS and ERDA as well as the increment in the width of spectra occurs,which corresponds to the change of stopping cross-section of helium atoms in the Ti film due to the change of physical-state of helium in the evolution of helium bubble.The ion beam analysis on the helium evolution is consistent with the THDS measurement.Ion beam technique opens interesting possibilities in the characterizing on the growth of helium bubbles.

  19. Cooling with Superfluid Helium

    CERN Document Server

    Lebrun, P

    2014-01-01

    The technical properties of helium II (‘superfluid’ helium) are presented in view of its applications to the cooling of superconducting devices, particularly in particle accelerators. Cooling schemes are discussed in terms of heat transfer performance and limitations. Large-capacity refrigeration techniques below 2 K are reviewed, with regard to thermodynamic cycles as well as process machinery. Examples drawn from existing or planned projects illustrate the presentation. Keywords: superfluid helium, cryogenics

  20. Proton Scattering on Liquid Argon

    Science.gov (United States)

    Bouabid, Ryan; LArIAT Collaboration

    2017-01-01

    LArIAT (Liquid Argon In A Test-beam) is a liquid argon time projection chamber (LArTPC) positioned in a charged particle beamline whose primary purpose is to study the response of LArTPC's to charged particle interactions. This previously unmeasured experimental data will allow for improvement of Monte Carlo simulations and development of identification techniques, important for future planned LArTPC neutrino experiments. LArIAT's beamline is instrumented to allow for the identification of specific particles as well as measurement of those particles' incoming momenta. Among the particles present in the beamline, the analysis presented here focuses on proton-Argon interactions. This study uses particle trajectories and calorimetric information to identify proton-Argon interaction candidates. We present preliminary data results on the measurement of the proton-Argon cross-section. Liquid Argon In A Test Beam. The work is my analysis made possible through the efforts of LArIAT detector, data, and software.

  1. Helium behaviour in implanted boron carbide

    Directory of Open Access Journals (Sweden)

    Motte Vianney

    2015-01-01

    Full Text Available When boron carbide is used as a neutron absorber in nuclear power plants, large quantities of helium are produced. To simulate the gas behaviour, helium implantations were carried out in boron carbide. The samples were then annealed up to 1500 °C in order to observe the influence of temperature and duration of annealing. The determination of the helium diffusion coefficient was carried out using the 3He(d,p4He nuclear reaction (NRA method. From the evolution of the width of implanted 3He helium profiles (fluence 1 × 1015/cm2, 3 MeV corresponding to a maximum helium concentration of about 1020/cm3 as a function of annealing temperatures, an Arrhenius diagram was plotted and an apparent diffusion coefficient was deduced (Ea = 0.52 ± 0.11 eV/atom. The dynamic of helium clusters was observed by transmission electron microscopy (TEM of samples implanted with 1.5 × 1016/cm2, 2.8 to 3 MeV 4He ions, leading to an implanted slab about 1 μm wide with a maximum helium concentration of about 1021/cm3. After annealing at 900 °C and 1100 °C, small (5–20 nm flat oriented bubbles appeared in the grain, then at the grain boundaries. At 1500 °C, due to long-range diffusion, intra-granular bubbles were no longer observed; helium segregates at the grain boundaries, either as bubbles or inducing grain boundaries opening.

  2. Formation and properties of metal clusters isolated in helium droplets.

    Science.gov (United States)

    Tiggesbäumker, Josef; Stienkemeier, Frank

    2007-09-14

    The unique conditions forming atomic and molecular complexes and clusters using superfluid helium nanodroplets have opened up an innovative route for studying the physical and chemical properties of matter on the nanoscale. This review summarizes the specific characteristics of the formation of atomic clusters partly generated far from equilibrium in the helium environment. Special emphasis is on the optical response, electronic properties as well as dynamical processes which are mostly affected by the surrounding quantum matrix. Experiments include the optical induced response of isolated cluster systems in helium under quite different excitation conditions ranging from the linear regime up to the violent interaction with a strong laser field leading to Coulomb explosion and the generation of highly charged atomic fragments. The variety of results on the outstanding properties in the quantum size regime highlights the peculiar capabilities of helium nanodroplet isolation spectroscopy.

  3. O(^3 p) Doped Helium Droplets

    Science.gov (United States)

    Brice, Joseph T.; Douberly, Gary E.

    2017-06-01

    Atomic oxygen (^3 P) is generated via thermolysis in a commerical thermal gas cracker (Mantis Ltd. MGC-75). Complexes with HCN were investigated to qualitatively assess the doping efficiency of O(^3 P) into a helium droplet. Theoretical calculations of a linear O \\cdot\\cdot\\cdot HCN (^3 Σ) complex at the CCSD(T)/aug-cc-pVTZ level are consistent with the rotational constants extracted from the rotational substructure in the experimental spectra, and with dipole moments approximated from Stark spectra. The thermal source will be used to study reactions between O(^3 P) and hydrocarbons in helium droplets, and preliminary data on this topic will be presented.

  4. Atomic transportation via carbon nanotubes.

    Science.gov (United States)

    Wang, Quan

    2009-01-01

    The transportation of helium atoms in a single-walled carbon nanotube is reported via molecular dynamics simulations. The efficiency of the atomic transportation is found to be dependent on the type of the applied loading and the loading rate as well as the temperature in the process. Simulations show the transportation is a result of the van der Waals force between the nanotube and the helium atoms through a kink propagation initiated in the nanotube.

  5. Vacuum ultraviolet radiation emitted by microwave driven argon plasmas

    Science.gov (United States)

    Espinho, S.; Felizardo, E.; Henriques, J.; Tatarova, E.

    2017-04-01

    Vacuum ultraviolet (VUV) radiation emitted by microwave driven argon plasmas has been investigated at low-pressure conditions (0.36 mbar). A classical surface-wave sustained discharge at 2.45 GHz has been used as plasma source. VUV radiation has been detected by emission spectroscopy in the 30-125 nm spectral range. The spectrum exhibits atomic and ionic argon emissions with the most intense spectral lines corresponding to the atomic resonance lines, at 104.8 nm and 106.7 nm, and to the ion lines, at 92.0 nm and 93.2 nm. Emissions at lower wavelengths were also detected, including lines with no information concerning level transitions in the well-known NIST database (e.g., the atomic line at 89.4 nm). The dependence of the lines' intensity on the microwave power delivered to the launcher was investigated. The electron density was estimated to be around 1012 cm-3 using the Stark broadening of the hydrogen Hβ line at 486.1 nm. The main population and loss mechanisms considered in the model for the excited argon atom and ion states emitting in the VUV range are discussed. The experimental results were compared to self-consistent model predictions, and a good agreement was obtained.

  6. Helium the disappearing element

    CERN Document Server

    Sears, Wheeler M

    2015-01-01

    The subject of the book is helium, the element, and its use in myriad applications including MRI machines, particle accelerators, space telescopes, and of course balloons and blimps. It was at the birth of our Universe, or the Big Bang, where the majority of cosmic helium was created; and stellar helium production continues. Although helium is the second most abundant element in the Universe, it is actually quite rare here on Earth and only exists because of radioactive elements deep within the Earth. This book includes a detailed history of the discovery of helium, of the commercial industry built around it, how the helium we actually encounter is produced within the Earth, and the state of the helium industry today. The gas that most people associate with birthday party balloons is running out. “Who cares?” you might ask. Well, without helium, MRI machines could not function, rockets could not go into space, particle accelerators such as those used by CERN could not operate, fiber optic cables would not...

  7. Effects of oxygen concentration on atmospheric pressure dielectric barrier discharge in Argon-Oxygen Mixture

    Science.gov (United States)

    Li, Xuechun; Li, Dian; Wang, Younian

    2016-09-01

    A dielectric barrier discharge (DBD) can generate a low-temperature plasma easily at atmospheric pressure and has been investigated for applications in trials in cancer therapy, sterilization, air pollution control, etc. It has been confirmed that reactive oxygen species (ROS) play a key role in the processes. In this work, we use a fluid model to simulate the plasma characteristics for DBD in argon-oxygen mixture. The effects of oxygen concentration on the plasma characteristics have been discussed. The evolution mechanism of ROS has been systematically analyzed. It was found that the ground state oxygen atoms and oxygen molecular ions are the dominated oxygen species under the considered oxygen concentrations. With the oxygen concentration increasing, the densities of electrons, argon atomic ions, resonance state argon atoms, metastable state argon atoms and excited state argon atoms all show a trend of decline. The oxygen molecular ions density is high and little influenced by the oxygen concentration. Ground state oxygen atoms density tends to increase before falling. The ozone density increases significantly. Increasing the oxygen concentration, the discharge mode begins to change gradually from the glow discharge mode to Townsend discharge mode. Project supported by the National Natural Science Foundation of China (Grant No. 11175034).

  8. Primary neutral helium in the heliosphere

    CERN Document Server

    Mueller, Hans-Reinhard

    2012-01-01

    Two years of neutral measurements by IBEX-Lo have yielded several direct observations of interstellar neutral helium and oxygen during preferred viewing seasons. Besides the interstellar signal, there are indications of the presence of secondary neutral helium and oxygen created in the heliosphere. Detailed modeling of these particle species is necessary to connect the measured fluxes to the pristine local interstellar medium while accounting for loss and production of neutral particles during their path through the heliosphere. In this contribution, global heliosphere models are coupled to analytic calculations of neutral trajectories to obtain detailed estimates of the neutral distribution function of primary interstellar helium atoms in the heliosphere, in particular in the inner heliosphere.

  9. Argon isotope fractionation induced by stepwise heating

    Science.gov (United States)

    Trieloff, Mario; Falter, Martina; Buikin, Alexei I.; Korochantseva, Ekaterina V.; Jessberger, Elmar K.; Altherr, Rainer

    2005-03-01

    Noble gas isotopes are widely used to elucidate the history of the rocks in which they have been trapped, either from distinct reservoirs or by accumulation following radioactive decay. To extract noble gases from their host rocks, stepwise heating is the most commonly used technique to deconvolve isotopically different components, e.g., atmospheric, in situ radiogenic, or excess radiogenic from mantle or crustal reservoirs. The accurate determination of the isotopic composition of these different components is of crucial importance, e.g., for ages obtained by 40Ar- 39Ar stepheating plateaus. However, diffusion theory-based model calculations predict that the stepwise thermal extraction process from mineral phases induces isotope fractionation and, hence, adulterates the original composition. Such effects are largely unconsidered, as they are small and a compelling experimental observation is lacking. We report the first unequivocal evidence for significant mass fractionation of argon isotopes during thermal extraction, observed on shungite, a carbon-rich Precambrian sedimentary rock. The degree of fractionation, as monitored by 38Ar/ 36Ar and 40Ar/ 36Ar ratios, very well agrees with theoretical predictions assuming an inverse square root dependence of diffusion coefficient and atomic mass, resulting in easier extraction of lighter isotopes. Hence, subatmospheric 40Ar/ 36Ar ratios obtained for argon extracted at low temperatures may not represent paleoatmospheric argon. Shungite argon resembles modern atmospheric composition, but constraints on the timing of trapping appear difficult to obtain, as shungites are multicomponent systems. In 40Ar- 39Ar stepwise heating, the isotope fractionation effect could cause systematic underestimations of plateau ages, between 0.15 and 0.4% depending on age, or considerably higher if samples contain appreciable atmospheric Ar. The magnitude of this effect is similar to the presently achieved uncertainties of this increasingly

  10. Production of stable, non-thermal atmospheric pressure rf capacitive plasmas using gases other than helium or neon

    Science.gov (United States)

    Park, Jaeyoung; Henins, Ivars

    2005-06-21

    The present invention enables the production of stable, steady state, non-thermal atmospheric pressure rf capacitive .alpha.-mode plasmas using gases other than helium and neon. In particular, the current invention generates and maintains stable, steady-state, non-thermal atmospheric pressure rf .alpha.-mode plasmas using pure argon or argon with reactive gas mixtures, pure oxygen or air. By replacing rare and expensive helium with more readily available gases, this invention makes it more economical to use atmospheric pressure rf .alpha.-mode plasmas for various materials processing applications.

  11. 基于原子晶体构型的高压固氩中的多体相互作用%Many-body interaction of highly compressed solid argon based on atomic crystal configuration

    Institute of Scientific and Technical Information of China (English)

    郑兴荣; 付云; 付文羽; 李向富; 李继弘

    2015-01-01

    X射线衍射实验显示固氩是面心立方( fcc)晶格结构,目前对晶体氩的研究只限于两体,三体以及四体相互作用势。本文利用多体展开方法和超分子单、双(三)重激发耦合簇理论(CCSD(T))对固氩fcc晶格结构的三体和四体的几何构型、几何参数、不同体积下所有三体和四体构型的势能以及各构型所占比例等几个方面进行了准确的量子化学计算。结果表明:所有三体构型中对总的三体势能贡献最大的是构型1、构型6、构型12和构型23;三体势及其交换部分和色散部分的计算结果与现有解析经验势在长程部分符合得非常好,但在短程部分有较小差异。所有的四体构形中对总的四体势能贡献最大的是构型1,构型2,构型4,构型5,构型7和构型8;四体势及其交换势部分和色散部分的计算结果尚无解析经验势可比较。利用这些特殊构型的相关数据并结合其它构型,可拟合出更准确的三体经验势函数及其参数,也为拟合四体经验势函数及其参数提供了重要的参考价值。%X-ray diffraction experiments shows that solid argon is a face-centered cubic crystal structure ( fcc structure). At present, crystal argon is studied involving two-, three- and four-body potentials. Using the many-body expansion method and the double cluster with full single and double excitations plus perturbative treatment of triples ( CCSD( T) ) , the properties of fcc structure for solid argon which include geometrical config-uration, geometrical parameters, potential energy of three- and four-body potentials and the proportion of all configurations at different volumes were accurately calculated. It is concluded that the configuration 1 , 6 , 12 and 23 play most important role in all three-body potential configurations. The calculation results of three-body po-tential, exchange potential and dispersion potential are in good agreement with the analytic experience

  12. Localized helium excitations in 4He_N-benzene clusters

    CERN Document Server

    Huang, P; Huang, Patrick

    2003-01-01

    We compute ground and excited state properties of small helium clusters 4He_N containing a single benzene impurity molecule. Ground-state structures and energies are obtained for N=1,2,3,14 from importance-sampled, rigid-body diffusion Monte Carlo (DMC). Excited state energies due to helium vibrational motion near the molecule surface are evaluated using the projection operator, imaginary time spectral evolution (POITSE) method. We find excitation energies of up to ~23 K above the ground state. These states all possess vibrational character of helium atoms in a highly anisotropic potential due to the aromatic molecule, and can be categorized in terms of localized and collective vibrational modes. These results appear to provide precursors for a transition from localized to collective helium excitations at molecular nanosubstrates of increasing size. We discuss the implications of these results for analysis of anomalous spectral features in recent spectroscopic studies of large aromatic molecules in helium clu...

  13. Evidence for Argon Content in Pure Oxygen from Thermal Data

    Science.gov (United States)

    Steur, Peter P. M.; Yang, Inseok; Pavese, Franco

    2017-02-01

    Since many years it is known that argon impurities in oxygen change the temperature of the oxygen triple point by +12 K{\\cdot }mol^{-1} (positive, while most impurities decrease the temperature) without any effect on the melting range of this transition, for the impurity concentrations usually encountered in nominally pure gases. It has been hypothesized that thermal measurements on the α -β solid-to-solid transition at 23.8 K or the β -γ solid-to-solid transition at 43.8 K may give reliable evidence regarding the argon content. However, such measurements require very long times for full completion of each transition (with prohibitive costs if liquid helium is used) and for the α -β solid-to-solid transition the heat pulse method cannot be applied reliably. The availability of closed-cycle refrigerators permits the first obstacle to be surmounted. The automatic system earlier developed at INRIM during the EU Multicells project and used extensively for the project on the isotopic effect in neon is perfectly suited for such measurements. Thus, the uncertainties of the temperature measurements are similar to those obtained previously (of the order of 0.1 mK or less). Three argon-in-oxygen mixtures were prepared gravimetrically and certified at KRISS, just as was previously done for the work on the neon isotopic compositions. Results of continuous-current measurements on the α -β solid-to-solid transition, along with the triple-point data obtained with the heat pulse method, are presented for one cell with a known doped argon content, to be compared with similar data from a cell with oxygen of very high purity. In addition, some preliminary data for the β -γ solid-to-solid transition are given. The measurements on the mixture with the highest argon content, about 1002 μmol{\\cdot } mol^{-1}, imply a (linear) sensitivity of (116 ± 7) K{\\cdot }mol^{-1} for the α -β transition. This sensitivity may be different at much lower argon contents, and follow

  14. Simulation of Helium Behaviour in Titanium Crystals Using Molecular Dynamics

    Institute of Scientific and Technical Information of China (English)

    WANG Jun; HOU Qing; SUN Tie-Ying; WU Zhong-Cheng; LONG Xing-Gui; WU Xing-Chun; LUO Shun-Zhong

    2006-01-01

    @@ The behaviour of helium in Ti crystals at 300 K has been investigated by means of the molecular dynamics. The study is focused on the influences of He-Ti interaction on the aggregation of helium atoms in the substrate. When a Born-Mayer potential is used to describe the He-Ti interaction, the He atoms are unable to cluster with each other due to the weak bridge barrier that cannot trap the helium atoms, Whereas using a He-Ti potential that is constructed by fitting the ab initio pairwise He-Ti potential, the clustering of He atoms can be observed. The results indicate that suitable He-Ti potential plays an important role in the formation of He clusters in metals.Moreover, it is noted that the shape of the formed He cluster is irregular, and the produced defect prefers to congregating on one side of the He cluster rather than spreading symmetrically around it.

  15. Argon metastable dynamics and lifetimes in a direct current microdischarge

    Science.gov (United States)

    Stefanović, Ilija; Kuschel, Thomas; Schröter, Sandra; Böke, Marc

    2014-09-01

    In this paper we study the properties of a pulsed dc microdischarge with the continuous flow of argon. Argon metastable lifetimes are measured by tunable diode laser absorption spectroscopy (TDLAS) and are compared with calculated values which yield information about excitation and de-excitation processes. By increasing the gas flow-rate about 5 times from 10 to 50 sccm, the Arm lifetime increases from 1 to 5 μs due to the reduction of metastable quenching with gas impurities. Optical emission spectroscopy reveals nitrogen and water molecules as the main gas impurities. The estimated N2 density [N2] = 0.1% is too low to explain the measured metastable lifetimes. Water impurity was found to be the main de-excitation source of argon metastable atoms due to high quenching coefficients. The water impurity level of [H2O] = 0.15% to 1% is sufficient to bring calculated metastable lifetimes in line with experiments. The maximum value of water content in the discharge compared to the argon atoms is estimated to approximately 6%, due to the large surface to volume ratio of the microdischarge. The current pulse releases the water molecules from the electrode surface and they are either re-adsorbed in the time between 0.4 ms for [H2O] = 1% and 2.6 ms for [H2O] = 0.15% or pumped out of the discharge with the speed equal to the gas flow-rate. Depending on its partial pressure, the water impurity re-adsorption time is of the order of magnitude or less then the argon gas residence time.

  16. Argon metastable dynamics and lifetimes in a direct current microdischarge

    Energy Technology Data Exchange (ETDEWEB)

    Stefanović, Ilija [Institute of Physics, University of Belgrade, Pregrevica 118, 11080 Belgrade (Serbia); Kuschel, Thomas; Schröter, Sandra; Böke, Marc [Ruhr-Universität Bochum, Institute for Experimental Physics II, Universitätsstraße 150, 44780 Bochum (Germany)

    2014-09-21

    In this paper we study the properties of a pulsed dc microdischarge with the continuous flow of argon. Argon metastable lifetimes are measured by tunable diode laser absorption spectroscopy (TDLAS) and are compared with calculated values which yield information about excitation and de-excitation processes. By increasing the gas flow-rate about 5 times from 10 to 50 sccm, the Ar{sup m} lifetime increases from 1 to 5 μs due to the reduction of metastable quenching with gas impurities. Optical emission spectroscopy reveals nitrogen and water molecules as the main gas impurities. The estimated N₂ density [N₂]=0.1% is too low to explain the measured metastable lifetimes. Water impurity was found to be the main de-excitation source of argon metastable atoms due to high quenching coefficients. The water impurity level of [H₂O]=0.15% to 1% is sufficient to bring calculated metastable lifetimes in line with experiments. The maximum value of water content in the discharge compared to the argon atoms is estimated to approximately 6%, due to the large surface to volume ratio of the microdischarge. The current pulse releases the water molecules from the electrode surface and they are either re-adsorbed in the time between 0.4 ms for [H₂O]=1% and 2.6 ms for [H₂O]=0.15% or pumped out of the discharge with the speed equal to the gas flow-rate. Depending on its partial pressure, the water impurity re-adsorption time is of the order of magnitude or less then the argon gas residence time.

  17. Coherence and Relaxation in Potassium-Doped Helium Droplets Studied by Femtosecond Pump-Probe Spectroscopy

    Science.gov (United States)

    Stienkemeier, F.; Meier, F.; Hägele, A.; Lutz, H. O.; Schreiber, E.; Schulz, C. P.; Hertel, I. V.

    1999-09-01

    Superfluid helium droplets are doped with potassium atoms to form complexes in which the metal atom is weakly bound to the cluster surface. The dynamics of these systems upon electronic excitation of the metal atom is probed by means of femtosecond pump-probe spectroscopy. Alignment of the excited potassium p orbital parallel to the cluster surface leads to quantum interferences, the decay of which gives information on the ultrafast perturbation of the induced atomic coherence by the superfluid environment; exciting the p state aligned perpendicularly, the strong repulsive interaction with the helium surface comes into play and the response of the helium environment is followed in time.

  18. Helium-Charged Titanium Films Deposited by Pulsed Laser Deposition in an Electron-Cyclotron-Resonance Helium Plasma Environment

    Institute of Scientific and Technical Information of China (English)

    金钦华; 胡佩钢; 凌浩; 吴嘉达; 施立群; 周筑颖

    2003-01-01

    Titanium thin films incorporated with helium are produced by pulsed laser deposition in an electron cyclotron resonance helium plasma environment. Helium is distributed evenly in the film and a relatively high He/Ti atomic ratio (~ 20%) is obtained from the proton backscattering spectroscopy. This high concentration ofhelium leads to a surface blistering which is observed by scanning electron microscopy. Laser repetition rate has little influence on film characters. Substrate bias voltage is also changed for the helium incorporating mechanism study, and this is a helium ion implantation process during the film growth. Choosing suitable substrate bias voltage, one can avoid the damage produced by ion implantation, which is always present in general implantation case.

  19. Effects of dark atom excitations

    CERN Document Server

    Cudell, Jean-René; Wallemacq, Quentin

    2014-01-01

    New stable quarks and charged leptons may exist and be hidden from detection, as they are bound by Coulomb interaction in neutral dark atoms of composite dark matter. This possibility leads to fundamentally new types of indirect effects related to the excitation of such dark atoms followed by their electromagnetic de-excitation. Stable -2 charged particles, bound to primordial helium in O-helium (OHe) atoms, represent the simplest model of dark atoms. Here we consider the structure of OHe atomic levels which is a necessary input for the indirect tests of such composite dark matter scenarios, and we give the spectrum of electromagnetic transitions from the levels excited in OHe collisions.

  20. Helium at White Dwarf Photospheric Conditions: Preliminary Laboratory Results

    Science.gov (United States)

    Schaeuble, M.; Falcon, R. E.; Gomez, T. A.; Winget, D. E.; Montgomery, M. H.; Bailey, J. E.

    2017-03-01

    We present preliminary results of an experimental study exploring helium at photospheric conditions of white dwarf stars. These data were collected at Sandia National Laboratories' Z-machine, the largest x-ray source on earth. Our helium results could have many applications ranging from validating current DB white dwarf model atmospheres to providing accurate He pressure shifts at varying temperatures and densities. In a much broader context, these helium data can be used to guide theoretical developments in new continuum-lowering models for two-electron atoms. We also discuss future applications of our updated experimental design, which enables us to sample a greater range of densities, temperatures, and gas compositions.

  1. Helium at white dwarf photospheric conditions: preliminary laboratory results

    CERN Document Server

    Schaeuble, Marc; Gomez, Thomas A; Winget, Don E; Montgomery, Michael H; Bailey, James E

    2016-01-01

    We present preliminary results of an experimental study exploring helium at photospheric conditions of white dwarf stars. These data were collected at Sandia National Laboratories' Z-machine, the largest x-ray source on earth. Our helium results could have many applications ranging from validating current DB white dwarf model atmospheres to providing accurate He pressure shifts at varying temperatures and densities. In a much broader context, these helium data can be used to guide theoretical developments in new continuum-lowering models for two-electron atoms. We also discuss future applications of our updated experimental design, which enables us to sample a greater range of densities, temperatures, and gas compositions.

  2. Advances in Helium Cryogenics

    Science.gov (United States)

    Sciver, S. W. Van

    This review provides a survey of major advances that have occurred in recent years in the area of helium cryogenics. Helium-temperature cryogenics is the enabling technology for a substantial and growing number of low-temperature systems from superconducting magnets to space-based experimental facilities. In recent years there have been many advances in the technology of low-temperature helium, driven mostly by new applications. However, to keep the review from being too broad, this presentation focuses mainly on three of the most significant advances. These are: (1) the development of large-scale recuperative refrigeration systems mainly for superconducting magnet applications in accelerators and other research facilities; (2) the use of stored superfluid helium (He II) as a coolant for spacebased astrophysics experiments; and (3) the application of regenerative cryocoolers operating at liquid helium temperatures primarily for cooling superconducting devices. In each case, the reader should observe that critical technologies were developed to facilitate these applications. In addition to these three primary advances, other significant helium cryogenic technologies are briefly reviewed at the end of this chapter, along with some vision for future developments in these areas.

  3. Molecular Dynamics Simulations of helium Behaviour in Copper Crystals

    Institute of Scientific and Technical Information of China (English)

    王玲; 宁西京

    2003-01-01

    Molecular dynamics simulations are performed to investigate the behaviour of helium atoms generated from tritium decay in perfect Cu crystals at 300K. At the early stage just after a 3He atom generation, the lattice structure is badly deformed and the local temperature rises considerably above 300 K. Single 3He atom diffuses by interstitial paths, whereas two 3He atoms attract each other and can form a stable dimer, which pushes a Cu atom out of its original lattice site and occupies the vacancy. This dimer can catch another 3He atom and form a trimer with an equilateral triangular structure.

  4. Cluster dynamics modeling of accumulation and diffusion of helium in neutron irradiated tungsten

    Energy Technology Data Exchange (ETDEWEB)

    Li, Y.G.; Zhou, W.H.; Huang, L.F. [Key Laboratory for Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei 230031 (China); Zeng, Z., E-mail: zzeng@theory.issp.ac.cn [Key Laboratory for Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei 230031 (China); Ju, X. [Department of Physics, University of Science and Technology Beijing, Beijing 100083 (China)

    2012-12-15

    A cluster dynamics model based on rate theory has been developed to study the accumulation and diffusion processes of helium in tungsten under synergistic effects of helium implantation and neutron irradiation. By including self-interstitial atoms, vacancies and helium atoms as well as their clusters and further using more reliable parameters, the evolution of different types of defects with time and depth is investigated. The calculated results are comparable with experiments. The cases of helium plasma corresponding to the first wall and to the divertor are taken into account. The accumulation and diffusion behaviors of helium in tungsten are illustrated by the time and depth dependence of helium concentration in tungsten with or without the neutron irradiation, the contribution of different types of helium clusters/complexes to helium concentration and the depth profiles of different mobile defects and helium-vacancy complexes. It is concluded that the competition of trapping and diffusion effects dominates the behavior of helium atoms in tungsten for these two typical cases. Understanding these mechanisms is important for estimating damages to the plasma-facing materials.

  5. Diffusion Monte Carlo calculation of rate of elastic transmission of a helium vapor beam through a slab of superfluid helium

    Science.gov (United States)

    Lutsyshyn, Y.; Halley, J. W.

    2011-01-01

    We present the results of diffusion Monte Carlo calculations of the elastic transmission of a low-energy beam of helium atoms through a suspended slab of superfluid helium. These calculations represent a significant improvement on variational Monte Carlo methods which were previously used to study this problem. The results are consistent with the existence of a condensate-mediated transmission mechanism, which would result in very fast transmission of pulses through a slab.

  6. Numerical investigation of depth profiling capabilities of helium and neon ions in ion microscopy

    Directory of Open Access Journals (Sweden)

    Patrick Philipp

    2016-11-01

    Full Text Available The analysis of polymers by secondary ion mass spectrometry (SIMS has been a topic of interest for many years. In recent years, the primary ion species evolved from heavy monatomic ions to cluster and massive cluster primary ions in order to preserve a maximum of organic information. The progress in less-damaging sputtering goes along with a loss in lateral resolution for 2D and 3D imaging. By contrast the development of a mass spectrometer as an add-on tool for the helium ion microscope (HIM, which uses finely focussed He+ or Ne+ beams, allows for the analysis of secondary ions and small secondary cluster ions with unprecedented lateral resolution. Irradiation induced damage and depth profiling capabilities obtained with these light rare gas species have been far less investigated than ion species used classically in SIMS. In this paper we simulated the sputtering of multi-layered polymer samples using the BCA (binary collision approximation code SD_TRIM_SP to study preferential sputtering and atomic mixing in such samples up to a fluence of 1018 ions/cm2. Results show that helium primary ions are completely inappropriate for depth profiling applications with this kind of sample materials while results for neon are similar to argon. The latter is commonly used as primary ion species in SIMS. For the two heavier species, layers separated by 10 nm can be distinguished for impact energies of a few keV. These results are encouraging for 3D imaging applications where lateral and depth information are of importance.

  7. Numerical investigation of depth profiling capabilities of helium and neon ions in ion microscopy.

    Science.gov (United States)

    Philipp, Patrick; Rzeznik, Lukasz; Wirtz, Tom

    2016-01-01

    The analysis of polymers by secondary ion mass spectrometry (SIMS) has been a topic of interest for many years. In recent years, the primary ion species evolved from heavy monatomic ions to cluster and massive cluster primary ions in order to preserve a maximum of organic information. The progress in less-damaging sputtering goes along with a loss in lateral resolution for 2D and 3D imaging. By contrast the development of a mass spectrometer as an add-on tool for the helium ion microscope (HIM), which uses finely focussed He(+) or Ne(+) beams, allows for the analysis of secondary ions and small secondary cluster ions with unprecedented lateral resolution. Irradiation induced damage and depth profiling capabilities obtained with these light rare gas species have been far less investigated than ion species used classically in SIMS. In this paper we simulated the sputtering of multi-layered polymer samples using the BCA (binary collision approximation) code SD_TRIM_SP to study preferential sputtering and atomic mixing in such samples up to a fluence of 10(18) ions/cm(2). Results show that helium primary ions are completely inappropriate for depth profiling applications with this kind of sample materials while results for neon are similar to argon. The latter is commonly used as primary ion species in SIMS. For the two heavier species, layers separated by 10 nm can be distinguished for impact energies of a few keV. These results are encouraging for 3D imaging applications where lateral and depth information are of importance.

  8. First measurement of helium on Mars: Implications for the problem of radiogenic gases on the terrestrial planets

    Science.gov (United States)

    Krasnopolsky, V. A.; Bowyer, S.; Chakrabarti, S.; Gladstone, G. R.; Mcdonald, J. S.

    1994-01-01

    108 +/- 11 photons of the martian He 584-A airglow detected by the Extreme Ultraviolet Explorer (EUVE) satellite during a 2-day exposure (January 22-23, 1993) correspond to the effective disk average intensity of 43 +/- 10 Rayleigh (Ra). Radiative transfer calculations, using a model atmosphere appropriate to the conditions of the observation and having an exospheric temperature of 210 +/- 20 K, result in a He mixing ratio of 1.1 +/- 0.4 ppm in the lower atmosphere. Nonthermal escape of helium is due to electron impact ionization and pickup of He(+) by the solar wind, to collisions with hot oxygen atoms, and to charge exchange with molecular species with corresponding column loss rates of 1.4 x 10(exp 5), 3 x 10(exp 4), and 7 x 10(exp 3)/sq cm/s, respectively. The lifetime of helium on Mars is 5 x 10(exp 4) years. the He outgassing rate, coupled with the Ar-40 atmospheric abundance and with the K:U:Th ratio measured in the surface rocks, is used as input to a single two-reservoir degassing model which is applied to Mars and then to Venus. A similar model with known abundances if K, U, and Th is applied to Earth. The models for Earth and Mars presume loss of all argon accumulated in the atmospheres during the first billion years by large-scale meteorite and planetesimal impacts. The models show that the degassing coefficients for all three planets may be approximated by function delta = delta(sub 0) x (t(sub 0)/t)(exp 1/2) with delta(sub 0) = 0.1, 0.04, and 0.0125 Byr for Earth, Venus, and Mars, respectively. After a R(exp 2) correction this means that outgassing processes on Venus and Mars are weaker than on Earth by factors of 3 and 30, respectively. Mass ratios of U and Th are almost the same for all three planets, while potassiumis depleted by a factor of 2 in Venus and Mars. Mass ratio of helium and argon are close to 5 x 10(exp -9) and 2 x 10(exp -8) g/g in the interiors of all three planets. The implications of these results are discussed.

  9. Behaviors of helium in vanadium:Stability, diffusion, vacancy trapping and ideal tensile strength

    Institute of Scientific and Technical Information of China (English)

    Lijiang Gui; Yuelin Liu; Weitian Wang; Yinan Liu; Kameel Arshad; Ying Zhang; Guanghong Lu; Junen Yao

    2013-01-01

    The behaviors of helium in vanadium including stability, diffusion, and its interaction with vacancy as well as its effects on the ideal tensile strength was investigated by a first-principles method. The activation energy barrier of helium was calculated to be 0.09 eV, which is consistent with the experimental result. The results indicated that the vacancy can lead to a directed helium segregation into the vacancy to form a helium cluster since the vacancy provides a “lower atomic and electron density region”as a large driving force for helium binding. It is easy for a mono-vacancy to trap helium and form a HenV complex. The first-principles computational tensile test demonstrates that helium obviously decreased the tensile strength of vanadium.

  10. Cosmic Ray Helium Hardening

    CERN Document Server

    Ohira, Yutaka

    2010-01-01

    Recent observations by CREAM, ATIC-2 and PAMELA experiments suggest that (1) the spectrum of cosmic ray (CR) helium is harder than that of CR proton below the knee $10^15 eV$ and (2) all CR spectra become hard at $\\gtrsim 10^{11} eV/n$. We propose a new picture that higher energy CRs are generated in more helium-rich region to explain the hardening (1) without introducing different sources for CR helium. The helium to proton ratio at $\\sim 100$ TeV exceeds the Big Bang abundance $Y=0.25$ by several times, and the different spectrum is not reproduced within the diffusive shock acceleration theory. We argue that CRs are produced in the chemically enriched region, such as a superbubble, and the outward-decreasing abundance naturally leads to the hard spectrum of CR helium when escaping from the supernova remnant (SNR) shock. We provide a simple analytical spectrum that also fits well the hardening (2) because of the decreasing Mach number in the hot superbubble with $\\sim 10^6$ K. Our model predicts hard and con...

  11. Liquid Argon Barrel Cryostat Arrived

    CERN Multimedia

    Pailler, P

    Last week the first of three cryostats for the ATLAS liquid argon calorimeter arrived at CERN. It had travelled for 46 days over several thousand kilometers from Japan to CERN. During three years it has been fabricated by Kawasaki Heavy Industries Ltd. at Harima, close to Kobe, under contract from Brookhaven National Laboratory (BNL) of the U.S.. This cryostat consists of two concentric cylinders made of aluminium: the outer vacuum vessel with a diameter of 5.5 m and a length of 7 m, and the inner cold vessel which will contain the electromagnetic barrel calorimeter immersed in liquid argon. The total weight will be 270 tons including the detectors and the liquid argon. The cryostat is now located in building 180 where it will be equipped with 64 feed-throughs which serve for the passage of 122,880 electrical lines which will carry the signals of the calorimeter. After integration of the calorimeter, the solenoidal magnet of ATLAS will be integrated in the vacuum vessel. A final cold test of the cryostat inc...

  12. Opacity measurements in shock-generated argon plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Erskine, D.

    1993-07-01

    Dense plasmas having uniform and constant density and temperature are generated by passage of a planar shock wave through gas. The opacity of the plasma is accurately measured versus wavelength by recording the risetime of emitted light. This technique is applicable to a wide variety of species and plasma conditions. Initial experiments in argon have produced plasmas with 2 eV temperatures, 0.004--0.04 g/cm{sup 3} densities, and coupling parameters {Gamma} {approximately}0.3--0.7. Measurements in visible light are compared with calculations using the HOPE code. An interesting peak in the capacity at 400 nm is observed for the first time and is identified with the 4s-5p transition in excited neutral argon atoms.

  13. Microwave Spectrum and Molecular Structure of the ARGON-CIS-1,2-DICHLOROETHYLENE Complex

    Science.gov (United States)

    Marshall, Mark D.; Leung, Helen O.; Nelson, Craig J.; Yoon, Leonard H.

    2016-06-01

    The non-planar molecular structure of the complex formed between the argon atom and cis-1,2-dichloroethylene is determined via analysis of its microwave spectrum. Spectra of the 35Cl and 37Cl isotopologues are observed in natural abundance and the nuclear quadrupole splitting due to the two chlorine nuclei is fully resolved. In addition, the complete quadrupole coupling tensor for the cis-1,2-dichloroethylene molecule, including the single non-zero off-diagonal element, has been determined. Unlike the argon-cis-1,2-difluoroethylene and the argon-vinyl chloride complexes, tunneling between the two equivalent non-planar configurations of argon-cis-1,2-dichloroethylene is not observed.

  14. A design for a pinhole scanning helium microscope

    Energy Technology Data Exchange (ETDEWEB)

    Barr, M.; Fahy, A. [Centre for Organic Electronics, University of Newcastle, Callaghan, NSW 2308 (Australia); Jardine, A.; Ellis, J.; Ward, D. [Cavendish Laboratory, University of Cambridge, Madingley Road, Cambridge CB3 0HE (United Kingdom); MacLaren, D.A. [Dept. of Physics, University of Glasgow, Glasgow G12 8QQ (United Kingdom); Allison, W. [Cavendish Laboratory, University of Cambridge, Madingley Road, Cambridge CB3 0HE (United Kingdom); Dastoor, P.C., E-mail: Paul.Dastoor@newcastle.edu.au [Centre for Organic Electronics, University of Newcastle, Callaghan, NSW 2308 (Australia)

    2014-12-01

    We present a simplified design for a scanning helium microscope (SHeM) which utilises almost entirely off the shelf components. The SHeM produces images by detecting scattered neutral helium atoms from a surface, forming an entirely surface sensitive and non-destructive imaging technique. This particular prototype instrument avoids the complexities of existing neutral atom optics by replacing them with an aperture in the form of an ion beam milled pinhole, resulting in a resolution of around 5 microns. Using the images so far produced, an initial investigation of topological contrast has been performed.

  15. Reactions of atomic cations with methane: gas phase room-temperature kinetics and periodicities in reactivity.

    Science.gov (United States)

    Shayesteh, Alireza; Lavrov, Vitali V; Koyanagi, Gregory K; Bohme, Diethard K

    2009-05-14

    Reactions of methane have been measured with 59 atomic metal cations at room temperature in helium bath gas at 0.35 Torr using an inductively-coupled plasma/selected-ion flow tube (ICP/SIFT) tandem mass spectrometer. The atomic cations were produced at approximately 5500 K in an ICP source and allowed to decay radiatively and to thermalize by collisions with argon and helium atoms prior to reaction. Rate coefficients and product distributions are reported for the reactions of fourth-row atomic cations from K(+) to Se(+), of fifth-row atomic cations from Rb(+) to Te(+) (excluding Tc(+)), of sixth-row atomic cations from Cs(+) to Bi(+), and of the lanthanide cations from La(+) to Lu(+) (excluding Pm(+)). Two primary reaction channels were observed: C-H bond insertion with elimination of H(2), and CH(4) addition. The bimolecular H(2) elimination was observed in the reactions of CH(4) with As(+), Nb(+), and some sixth-row metal cations, i.e., Ta(+), W(+), Os(+), Ir(+), Pt(+); secondary and higher-order H(2) elimination was observed exclusively for Ta(+), W(+), and Ir(+) ions. All other transition-metal cations except Mn(+) and Re(+) were observed to react with CH(4) exclusively by addition, and up to two methane molecules were observed to add sequentially to most transition-metal ions. CH(4) addition was also observed for Ge(+), Se(+), La(+), Ce(+), and Gd(+) ions, while the other main-group and lanthanide cations did not react measurably with methane.

  16. Composing Experimental Environment of PRIDE Argon cell

    Energy Technology Data Exchange (ETDEWEB)

    Noh, Seonho; Jang, Yongkuk; Cho, Il Je [Korea Atomic Energy Research Institute, Daejeon (Korea, Republic of)

    2015-10-15

    In PRIDE depleted Uranium feed material and a depleted Uranium mixed with some surrogate material are used for performing engineering scale Pyroprocessing. PRIDE has to maintain inert atmosphere because of the characteristic of Electrolytic Reduction technology, Electro refining technology, Electrowinning technology. The impurity concentration of the Argon cell has to be under 50 ppm(Oxygen, moisture). Atmospheric pressure changes and temperature changes can affect the Argon cell's impurity concentration. In this paper, how to compose the Argon cell impurity concentration under 50 ppm to make the exact optimal experimental environment(Oxygen, moisture) will be introduced. Composing the exact optimal experimental environment by supplying Argon gas have been introduced in this paper. Continuously supplying Argon gas which is heavier than the Oxygen through the bottom of the Argon cell the oxygen eventually discharged through the high vent fan and lower the impurity concentration of Oxygen.

  17. 氩氦刀冷冻消融联合TACE治疗巨大肝癌的临床观察∗%Clinical observation of argon-helium knife cryotherapy combined with transcatheter arterial chemoemboli-zation (TACE) on huge liver cancer

    Institute of Scientific and Technical Information of China (English)

    邱国钦; 许丽贞; 罗鹏飞; 陈玉强

    2015-01-01

    Objective To explore the efficacy and safety of argon⁃helium knife cryotherapy combined with transcatheter arte⁃rial chemoembolization ( TACE) on huge hepatocellular carcinoma. Methods Eighty⁃five patients with huge liver cancer from Septem⁃ber 2006 to August 2011 were analyzed retrospectively. Observation group ( n=44) received one to two TACE and one to three argon⁃helium knife cryotherapy after one month sequently, while the control group ( n=41) received TACE treatment only. Response to chemotherapy was assessed by RECIST criteria 1. 0 and follow⁃up data was investigated. Results The response rate of observation group was 70. 5%, higher than 46. 3% of the control group (P<0. 05). The 1⁃, 2⁃, 3⁃year survival rates of observation group were 77. 3%, 56. 8% and 36. 4%, and medium overall survival time was 19. 2 months, which were all higher than the 51. 2%, 36. 6%, 14. 6% and 11. 8 months of control group ( P<0. 05) . The adverse reaction of both groups were mild⁃to⁃moderate and tolerable. Con⁃clusion Argon⁃helium knife cryotherapy combined with TACE has synergism effect and minimally invasive, and provide a new regiem for comprehensive treatment on huge hepatocellular carcinoma.%目的:探讨氩氦刀冷冻消融联合经肝动脉化疗栓塞( TACE)治疗巨大肝癌的有效性和安全性。方法回顾性分析本院2006年9月至2011年8月收治的巨大肝癌患者85例,其中观察组44例先行1~2次TACE,1个月后序贯氩氦刀治疗1~3次,而对照组41例仅行单纯TACE治疗。按照实体瘤的疗效评价标准( RECIST)1.0版评价疗效并随访生存。结果观察组有效率( RR)为70.5%,高于对照组的46.3%( P<0.05);观察组1、2和3年生存率分别为77.3%、56.8%和36.4%,中位生存时间为19.2个月,均高于对照组的51.2%、36.6%、14.6%和11.8个月( P<0.05);两组患者的不良反应均为轻中度且可耐受。

  18. The clinical application of CT-guided argon-helium cryoablation combined with 125 I radioactive particle in treating liver cancer located under the diaphragm%CT 导引下氩氦冷冻消融联合125I 放射粒子植入治疗膈顶部肝癌的临床应用

    Institute of Scientific and Technical Information of China (English)

    左太阳; 杨卫国; 张忠涛; 咸利军; 张秀亮; 马群; 王松

    2015-01-01

    Objective To evaluate the method of CT‐guided argon‐helium cryoablation combined with 125 I radioactive particle in treating liver cancer located under the diaphragm and to discuss the efficacy of this technique .Methods We se‐lected 16 cases of liver cancer located under the diaphragm .All the cases had been diagnosed by 3‐stage CT scanning and confirmed pathologically .The cancer had been treated by argon‐helium cryoablation combined with 125 I radioactive parti‐cle .Results The rate of the decline in serum AFP level and the efficiency after 3‐ ,6‐ ,12‐ ,24‐month treatment were 100% (16/16) ,100% (16/16) ,93 .8% (15/16) ,87 .5% (14/16) and 100% (16/16) ,100% (16/16) ,87 .5% (14/16) , 87.5% (14/16) .The 3‐ ,6‐ ,12‐ ,24‐month survival rates were 100% (16/16) ,100% (16/16) ,100% (16/16) ,93 .8%(15/16) .Conclusion CT‐guided argon‐helium cryoablation combined with 125 I radioactive particle in treating liver cancer located under the diaphragm is an efficient method for increasing the part control and survival rate for liver cancer located under the diaphragm .%目的:探讨 CT 引导下氩氦冷冻消融联合125 I 放射粒子治疗膈顶部肝癌的方法、疗效。方法选择通过3期CT 增强扫描并经穿刺活检病理证实的膈顶部肝癌16例,行 CT 导引下氩氦冷冻消融联合125 I 放射粒子治疗。结果16例膈顶部肝癌患者治疗后3个月、6个月、12个月、24个月 AFP 下降率依次是100%(16/16),100%(16/16),93.8%(15/16),87.5%(14/16),肿瘤局部控制率依次是100%(16/16),100%(16/16),87.5%(14/16),87.5%(14/16)。结论 CT引导下氩氦冷冻消融联合125 I 放射粒子治疗膈顶部肝癌,疗效可靠,是提高治疗局部控制率和生存率的有效方法。

  19. Communication: Barium ions and helium nanodroplets: solvation and desolvation.

    Science.gov (United States)

    Zhang, Xiaohang; Drabbels, Marcel

    2012-08-07

    The solvation of Ba(+) ions created by the photoionization of barium atoms located on the surface of helium nanodroplets has been investigated. The excitation spectra corresponding to the 6p (2)P(1/2) ← 6s (2)S(1/2) and 6p (2)P(3/2) ← 6s (2)S(1/2) transitions of Ba(+) are found to be identical to those recorded in bulk He II [H. J. Reyher, H. Bauer, C. Huber, R. Mayer, A. Schafer, and A. Winnacker, Phys. Lett. A 115, 238 (1986)], indicating that the ions formed at the surface of the helium droplets become fully solvated by the helium. Time-of-flight mass spectra suggest that following the excitation of the solvated Ba(+) ions, these are being ejected from the helium droplets either as bare Ba(+) ions or as small Ba(+)He(n) (n < 20) complexes.

  20. Suicidal asphyxiation by using helium – two case reports

    Directory of Open Access Journals (Sweden)

    Anna Smędra

    2015-05-01

    Full Text Available Helium is one of inert gases causing physical asphyxiation, whose excess content in the breathing atmosphere reduces the partial pressure of oxygen and may be fatal after short-term exposure. When breathing a mixture of an inert gas (helium, nitrogen, argon with a small amount of oxygen, with the possibility of exhaling carbon dioxide, no warning signs characteristic of suffocation are perceived by the subject. Freedom from discomfort and pain, effectiveness, rapid effect and relatively easy availability of required accessories have resulted in the use of inert gases for suicidal purposes. The paper reports two cases of suicide committed by using a special kit consisting of the so-called “suicide bag” (or “exit bag” filled with helium supplied through a plastic tube. In both cases, examination of the sites where the corpses were found and analysis of collected material allowed to establish that before their death the subjects had searched the Internet for instructions on how to commit suicide using helium. Due to the advanced putrefaction process, the autopsies failed to determine the causes of their death unequivocally. However, the circumstances surrounding the deaths suggested rapid asphyxiation as a result of oxygen deficiency in the breathing mixture. Since in cases of the type discussed here the cause of death cannot generally be established by autopsy, knowledge of the circumstances of disclosure of the corpse, as well as examination of the cadaver and the death scene is of utmost importance.

  1. Generation of stable and low-divergence 10-MeV quasimonoenergetic electron bunch using argon gas jet

    Directory of Open Access Journals (Sweden)

    M. Mori

    2009-08-01

    Full Text Available The pointing stability and divergence of a quasimonoenergetic electron bunch generated in a self-injected laser-plasma acceleration regime using 4 TW laser is studied. A pointing stability of 2.4 mrad root-mean-square (rms and a beam divergence of 10.6 mrad (rms were obtained using an argon gas-jet target for 50 sequential shots, while these values were degraded by a factor of 3 at the optimum condition using helium. The peak electron energies were 8.5±0.7 and 24.8±3.6  MeV using argon and helium, respectively. The experimental results indicate that the different propagation condition could be generated with the different material, although it is performed with the same irradiation condition.

  2. Microwave Spectra and Molecular Structures of 2-CHLORO-1,1-DIFLUOROETHYLENE and its Complex with Argon

    Science.gov (United States)

    Messinger, Joseph P.; Knowlton, Gregory S.; Sundheim, Kathryn M.; Leung, Helen O.; Marshall, Mark D.

    2013-06-01

    Chirped-pulse and Balle-Flygare spectrometers are used to obtain Fourier transform microwave spectra of 2-chloro-1,1-difluoroethylene and its complex with argon from 5.5 to 21.0 GHz, allowing for the geometries of both species to be determined. A total of six isotopologues are observed each for the monomer and dimer, including the most abundant species, the singly-substituted ^{37}Cl and two singly-substituted ^{13}C isotopologues in natural abundance, and deuterated versions of both the ^{35}Cl and ^{37}Cl species using an isotopically enriched sample. Similar to the previously studied argon-haloethylene complexes, the argon shows a preference for close contact with heavier atoms. Tunneling of the argon between two equivalent non-planar structures, similar to that in argon-cis-1,2-difluoroethylene, is not observed in this complex.

  3. Improved hybrid Monte Carlo-fluid model for the electrical characteristics in an analytical radio-frequency glow discharge in argon

    NARCIS (Netherlands)

    Bogaerts, A.; Gijbels, R.; W. Goedheer,

    2001-01-01

    An improved hybrid Monte Carlo-fluid model for electrons, argon ions and fast argon atoms, is presented for the rf Grimm-type glow discharge. In this new approach, all electrons, including the large slow electron group in the bulk plasma, are treated with the Monte Carlo model. The calculation

  4. Broken symmetry makes helium

    CERN Multimedia

    Gray, P L

    2003-01-01

    "The subatomic pion particle breaks the charge symmetry rule that governs both fusion and decay. In experiments performed at the Indiana University Cyclotron Laboratory, physicists forced heavy hydrogen (1 proton + 1 neutron) to fuse into helium in a controlled, measurable environment" (1 paragraph).

  5. The scintillation of liquid argon

    CERN Document Server

    Heindl, T; Hofmann, M; Krücken, R; Oberauer, L; Potzel, W; Wieser, J; Ulrich, A

    2015-01-01

    A spectroscopic study of liquid argon from the vacuum ultraviolet at 110 nm to 1000 nm is presented. Excitation was performed using continuous and pulsed 12 keV electron beams. The emission is dominated by the analogue of the so called 2nd excimer continuum. Various additional emission features were found. The time structure of the light emission has been measured for a set of well defined wavelength positions. The results help to interpret literature data in the context of liquid rare gas detectors in which the wavelength information is lost due to the use of wavelength shifters.

  6. Structural determination of argon trimer

    Directory of Open Access Journals (Sweden)

    Xiguo Xie

    2015-09-01

    Full Text Available Rare gas clusters are model systems to investigate structural properties at finite size. However, their structures are difficult to be determined with available experimental techniques because of the strong coupling between the vibration and the rotation. Here we experimentally investigated multiple ionization and fragmentation dynamics of argon trimer by ultrashort intense laser fields and reconstructed their structures with Coulomb explosion technique. The measured structure distribution was compared with our finite-temperature ab initio calculations and the discrepancy was discussed. The present study provides a guidance for the development of theoretical methods for exploring the geometric structure of rare gas clusters.

  7. Helium segregation on surfaces of plasma-exposed tungsten.

    Science.gov (United States)

    Maroudas, Dimitrios; Blondel, Sophie; Hu, Lin; Hammond, Karl D; Wirth, Brian D

    2016-02-17

    We report a hierarchical multi-scale modeling study of implanted helium segregation on surfaces of tungsten, considered as a plasma facing component in nuclear fusion reactors. We employ a hierarchy of atomic-scale simulations based on a reliable interatomic interaction potential, including molecular-statics simulations to understand the origin of helium surface segregation, targeted molecular-dynamics (MD) simulations of near-surface cluster reactions, and large-scale MD simulations of implanted helium evolution in plasma-exposed tungsten. We find that small, mobile He n (1⩽  n  ⩽  7) clusters in the near-surface region are attracted to the surface due to an elastic interaction force that provides the thermodynamic driving force for surface segregation. This elastic interaction force induces drift fluxes of these mobile He n clusters, which increase substantially as the migrating clusters approach the surface, facilitating helium segregation on the surface. Moreover, the clusters' drift toward the surface enables cluster reactions, most importantly trap mutation, in the near-surface region at rates much higher than in the bulk material. These near-surface cluster dynamics have significant effects on the surface morphology, near-surface defect structures, and the amount of helium retained in the material upon plasma exposure. We integrate the findings of such atomic-scale simulations into a properly parameterized and validated spatially dependent, continuum-scale reaction-diffusion cluster dynamics model, capable of predicting implanted helium evolution, surface segregation, and its near-surface effects in tungsten. This cluster-dynamics model sets the stage for development of fully atomistically informed coarse-grained models for computationally efficient simulation predictions of helium surface segregation, as well as helium retention and surface morphological evolution, toward optimal design of plasma facing components.

  8. STIRAP on helium: Excitation to Rydberg states

    Science.gov (United States)

    Yuan, Deqian

    Research in optically induced transitions between dierent atomic levels has a long history. For transitions between states driven by a coherent optical eld, the theoretical eciency could be ideally high as 100% but there could be many factors preventing this. In the three state helium atom excitation process, i.e. 23S→33P→nL , the stimulated emission from intermediate state makes it hard to achieve ecient population transfer to the nal state through an intuitive excitation order. One technique to achieve a higher eciency is Stimulated Raman Adiabatic Passage (STIRAP) which is being studied and under research in our lab. Unlike traditional three level excitation processes, STIRAP actually uses a counter intuitive pulsed laser beams timing arrangement. The excitation objects are metastable helium atoms traveling in a vacuum system with a longitudinal velocity of ~ 1070 m/s. We are using a 389 nm UV laser to connect the 23S and the 33P state and a frequency tunable ~790 nm IR laser to connect the 33P state and the dierent Rydberg states. A third 1083 nm wavelength laser beam drives the 23S → 23P transition to transversely separate the residual metastable atoms and the Rydberg atoms for eciency measurements. The data is taken by a stainless steel detector in the vacuum system. As the Rydberg atoms will get ionized by blackbody radiation under room temperature, we can utilize this for their detection. An ion detector sitting on the eld plate is capable to collect the ion signals of the Rydberg atoms for detection. So far the whole system has not been ready for data collection and measurement, so here we are using data and results from previous theses for discussions. The highest transition frequency that has ever been achieved in our lab is around 70% after corrections.

  9. Measurement of helium production cross sections of iron for d-T neutrons by helium accumulation method

    Energy Technology Data Exchange (ETDEWEB)

    Takao, Yoshiyuki; Kanda, Yukinori; Nagae, Koji; Fujimoto, Toshihiro [Kyushu Univ., Fukuoka (Japan); Ikeda, Yujiro

    1997-03-01

    Helium production cross sections of Iron were measured by helium accumulation method for neutron energies from 13.5 to 14.9 MeV. Iron samples were irradiated with FNS, an intense d-T neutron source of JAERI. As the neutron energy varies according to the emission angle at the neutron source, the samples were set around the neutron source and were irradiated by neutrons of different energy depending on each sample position. The amount of helium produced in a sample was measured by Helium Atoms Measurement System at Kyushu University. The results of this work are in good agreement with other experimental data in the literature and also compared with the evaluated values in JENDL-3. (author)

  10. Nonradiative formation of the positron-helium triplet bound state

    Science.gov (United States)

    di Rienzi, Joseph; Drachman, Richard J.

    2007-02-01

    We have previously calculated the cross section for radiative formation of the interesting bound state consisting of a positron bound to helium, where the atomic electrons are in the triplet spin state. That process uses the metastable triplet helium system as target, and, as expected, it has a very small cross section. In this paper we examine a more probable process in which the state of interest is produced in an exchange rearrangement collision between a positronium atom and the singlet helium ground state: Ps+He(Se1)→PsHe+(Se3)+e- . The present calculation is done in the plane-wave Born approximation, using simple initial and final wave functions and compares post and prior forms.

  11. Kinetic modeling of the Townsend breakdown in argon

    Science.gov (United States)

    Macheret, S. O.; Shneider, M. N.

    2013-10-01

    Kinetic modeling of the Townsend breakdown in argon was performed in the "forward-back" approximation. The kinetic model was found to adequately describe the left branch of the Paschen curve, and the important role of ionization by fast ions and atoms near the cathode, as well as the increase in secondary emission coefficient in strong electric fields described in the literature, was confirmed. The modeling also showed that the electron energy distribution function develops a beam of high-energy electrons and that the runaway effect, i.e., the monotonic increase of the mean electron energy with the distance from the cathode, occurs at the left branch of the Paschen curve.

  12. Argon purge gas cooled by chill box

    Science.gov (United States)

    Spiro, L. W.

    1966-01-01

    Cooling argon purge gas by routing it through a shop-fabricated chill box reduces charring of tungsten inert gas torch head components. The argon gas is in a cooled state as it enters the torch and prevents buildup of char caused by the high concentrations of heat in the weld area during welding operations.

  13. Collisional-Radiative Modeling of Free-Burning Arc Plasma in Argon

    Science.gov (United States)

    2013-06-01

    7) For the radiative transitions, data recommended by Wiese et al. [30] is used. The transition probabilities Amn (s -1...Atoms and Molecules, Published in the 20th Century: Argon, Rep. NIFS-DATA-72, National Institute for Fusion Science (Jpn), 2003. [30] W. L. Wiese , J

  14. Low energy (e,2e) ionization of Argon in the equal energy sharing geometry

    CERN Document Server

    Mazevet, S; Langlois, J M; Tweed, R J; Robaux, O; Tannous, C; Fakhreddine, K

    2002-01-01

    Quantum Defect theory is a well established theoretical concept in modern spectroscopy. We show that this approach is useful in electron impact ionization problems where state of the art theoretical methods are presently restricted mostly to simple atomic targets. For the well documented Argon ionization case in equal energy sharing geometry the approach suggested leads to significant improvements compared to previous calculations.

  15. Atoms, molecules & elements

    CERN Document Server

    Graybill, George

    2007-01-01

    Young scientists will be thrilled to explore the invisible world of atoms, molecules and elements. Our resource provides ready-to-use information and activities for remedial students using simplified language and vocabulary. Students will label each part of the atom, learn what compounds are, and explore the patterns in the periodic table of elements to find calcium (Ca), chlorine (Cl), and helium (He) through hands-on activities.

  16. Helium mobility in SON68 borosilicate nuclear glass: A nuclear reaction analysis approach

    Energy Technology Data Exchange (ETDEWEB)

    Bès, R., E-mail: rene.bes@cnrs-orleans.fr [CNRS, UPR3079 CEMHTI, 1D Avenue de la Recherche Scientifique, 45071 Orléans cedex 2 (France); Sauvage, T. [CNRS, UPR3079 CEMHTI, 1D Avenue de la Recherche Scientifique, 45071 Orléans cedex 2 (France); Université d’Orléans, Faculté des Sciences, Avenue du Parc Floral, BP 6749, 45067 Orléans cedex 2 (France); Peuget, S. [CEA/DEN/VRH/DTCD/SECM/LMPA Marcoule (France); Haussy, J. [CEA, DAM, DIF, F-91297 Arpajon (France); Chamssedine, F. [Université Libanaise, Faculté des Sciences V, Nabatiyeh (Lebanon); Oliviero, E. [CSNSM, CNRS/IN2P3 and Université Paris-Sud, Bât. 104-108, F-91405 Orsay (France); Fares, T. [CEA/DEN/VRH/DTCD/SECM/LMPA Marcoule (France); Vincent, L. [Institut d’Electronique Fondamentale, CNRS and Université Paris-Sud, UMR 8622, F-91405 Orsay (France)

    2013-11-15

    The {sup 3}He behavior in the non active R7T7 type borosilicate glass called SON68 has been investigated using the implantation method to introduce helium in the material. Nuclear Reaction Analysis (NRA) was performed to follow the helium concentration depth profile evolution as a function of annealing time and temperature. In addition, in situ Transmission Electron Microscopy (TEM) has been implemented to study the formation of helium bubbles during both implantation and annealing processes. Numerical modeling with two different approaches is proposed and discussed to investigate the helium mobility mechanisms. Our study reveals for helium incorporation by implantation at low temperature the presence of several helium populations with disparate diffusivities. The most mobile helium fraction would be attributed to atomic diffusion. The corresponding activation energy value (0.61 eV) extracted from Arrhenius graphs is in good agreement with literature data. The results also highlight that the damages associated to helium sursaturation are the source of small helium clusters formation, with a reduced mobility instead of the atomic mobility measured by the infusion technique. Small cavities that support this assumption have been observed by TEM at low temperature.

  17. On the ground state of a model for compressed helium

    NARCIS (Netherlands)

    Seldam, C.A. ten; Groot, S.R. de

    1952-01-01

    In the problem of the “compressed helium atom”, the boundary condition that the wave function ψ must vanish at infinity (r = ∞), is replaced by: ψ = 0 at a finite r = r0. This problem is solved by a variational method, which for the limiting case of the free atom (r0 → ∞) coincides with one of Hylle

  18. Experimental studies of amplification using evaporation and adsorption of helium

    Energy Technology Data Exchange (ETDEWEB)

    More, T. [Brown Univ., Providence, RI (United States). Dept. of Physics; Adams, J.S. [Brown Univ., Providence, RI (United States). Dept. of Physics; Bandler, S.R. [Brown Univ., Providence, RI (United States). Dept. of Physics; Brouer, S.M. [Brown Univ., Providence, RI (United States). Dept. of Physics; Lanou, R.E. [Brown Univ., Providence, RI (United States). Dept. of Physics; Maris, H.J. [Brown Univ., Providence, RI (United States). Dept. of Physics; Seidel, G.M. [Brown Univ., Providence, RI (United States). Dept. of Physics

    1996-02-11

    The design of a phonon amplifier based on the evaporation of helium atoms from a superfluid film and their adsorption onto a bare solid surface is discussed. Experimental results indicate that substantial improvement in efficiency is required to be able to construct such an amplifier. A possible modification to achieve this improvement is considered. (orig.).

  19. On the shear strength of tungsten nano-structures with embedded helium

    Science.gov (United States)

    Smirnov, R. D.; Krasheninnikov, S. I.

    2013-08-01

    Modification of plastic properties of tungsten nano-structures under shear stress load due to embedded helium atoms is studied using molecular dynamics modelling. The modelling demonstrates that the yield strength of tungsten nano-structures reduces significantly with increasing embedded helium concentration. At high helium concentrations (>10 at%), the yield strength decreases to values characteristic to the pressure in helium nano-bubbles, which are formed in tungsten under such conditions and thought to be responsible for the formation of nano-fuzz on tungsten surfaces irradiated with helium plasma. It is also shown that tungsten plastic flow strongly facilitates coagulation of helium clusters to larger bubbles. The temperature dependencies of the yield strength are obtained.

  20. Education in Helium Refrigeration

    Science.gov (United States)

    Gistau Baguer, G. M.

    2004-06-01

    On the one hand, at the end of the time I was active in helium refrigeration, I noticed that cryogenics was stepping into places where it was not yet used. For example, a conventional accelerator, operating at room temperature, was to be upgraded to reach higher particle energy. On the other hand, I was a little bit worried to let what I had so passionately learned during these years to be lost. Retirement made time available, and I came gradually to the idea to teach about what was my basic job. I thought also about other kinds of people who could be interested in such lessons: operators of refrigerators or liquefiers who, often by lack of time, did not get a proper introduction to their job when they started, young engineers who begin to work in cryogenics… and so on. Consequently, I have assembled a series of lessons about helium refrigeration. As the audiences have different levels of knowledge in the field of cryogenics, I looked for a way of teaching that is acceptable for all of them. The course is split into theory of heat exchangers, refrigeration cycles, technology and operation of main components, process control, and helium purity.

  1. Effect of boundary conditions on the kinetics of helium release from structural materials

    Science.gov (United States)

    Zaluzhnyi, A. G.

    2015-11-01

    Gaseous products of nuclear reactions (specifically, helium) play a significant part in altering the material properties upon irradiation. It is known that atoms of inert gases promote the generation and growth of pores in irradiated materials and affect phenomena such as swelling, high-temperature irradiation embrittlement, etc. Therefore, a study of the behavior of helium (its production, accumulation, retention, and release) within structural materials is fairly topical. In order to validate the methods of express imitation of accumulation and retention of helium within structural materials under reactor irradiation, we perform a comparative analysis of the spectra of the rate of gas release from samples of austenitic steel 0Kh16N15M3B that were saturated with helium in different ways, i.e., through irradiation in a cyclotron, a magnetic massseparation setup, the IRT-2000 reactor, the BOR-60 reactor, and using the so-called tritium trick technique. The effect of the presence of dislocations and grain boundaries on the release of helium from materials is evaluated. The results of the research conducted show that the kinetics of helium release from samples saturated with helium through the bombardment with alpha particles of different energies, which ensures the simultaneous introduction of helium and radiation defects (in wide ranges of helium concentration and radiation damage) into the material lattice, is similar to the kinetics of helium release from samples irradiated in reactors.

  2. Helium anion formation inside helium droplets

    Science.gov (United States)

    Maalouf, Elias Jabbour Al; Reitshammer, Julia; Ribar, Anita; Scheier, Paul; Denifl, Stephan

    2016-07-01

    The formation of He∗- is examined with improved electron energy resolution of about 100 meV utilizing a hemispherical electron monochromator. The work presented provides a precise determination of the three previously determined resonance peak positions that significantly contribute to the formation of He∗- inside helium nanodroplets in the energy range from 20 eV to 29.5 eV. In addition, a new feature is identified located at 27.69 ± 0.18 eV that we assign to the presence of O2 as a dopant inside the droplet. With increasing droplet size a small blue shift of the resonance positions is observed. Also for the relatively low electron currents used in the present study (i.e., 15-70 nA) a quadratic dependence of the He∗- ion yield on the electron current is observed. Contribution to the Topical Issue "Advances in Positron and Electron Scattering", edited by Paulo Limao-Vieira, Gustavo Garcia, E. Krishnakumar, James Sullivan, Hajime Tanuma and Zoran Petrovic.

  3. Suspension of superfluid helium using cesium-coated surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Williams, M.C.; Giese, C.F.; Halley, J.W. [School of Physics and Astronomy, University of Minnesota, Minneapolis, Minnesota 55455 (United States)

    1996-03-01

    We report results of an experiment which demonstrates that a layer of superfluid helium can be suspended over a cesium-coated orifice. By measuring the layer thickness with a capacitance bridge, we have shown in two runs that fluid layers up to 2 mm thick were suspended over a 70-{mu}m-diam cesium-coated orifice in a platinum foil for over 2 h in a cryostat held at 1.2 K. The effect depends on the recently established fact that superfluid helium does not wet cesium-coated surfaces. As a consequence, superfluid helium is expected to form a stable meniscus across such a cesium-coated hole. The observed depths of suspended helium are consistent with a simple theoretical model based on this picture. We briefly discuss the possible application of this method to the performance of a proposed experiment to study quantum coherence in superfluid helium by directing pulsed beams of helium atoms at such a suspended layer of fluid. {copyright} {ital 1996 The American Physical Society.}

  4. Helium effects on microstructural change in RAFM steel under irradiation: Reaction rate theory modeling

    Science.gov (United States)

    Watanabe, Y.; Morishita, K.; Nakasuji, T.; Ando, M.; Tanigawa, H.

    2015-06-01

    Reaction rate theory analysis has been conducted to investigate helium effects on the formation kinetics of interstitial type dislocation loops (I-loops) and helium bubbles in reduced-activation-ferritic/martensitic steel during irradiation, by focusing on the nucleation and growth processes of the defect clusters. The rate theory model employs the size and chemical composition dependence of thermal dissociation of point defects from defect clusters. In the calculations, the temperature and the production rate of Frenkel pairs are fixed to be T = 723 K and PV = 10-6 dpa/s, respectively. And then, only the production rate of helium atoms was changed into the following three cases: PHe = 0, 10-7 and 10-5 appm He/s. The calculation results show that helium effect on I-loop formation quite differs from that on bubble formation. As to I-loops, the loop formation hardly depends on the existence of helium, where the number density of I-loops is almost the same for the three cases of PHe. This is because helium atoms trapped in vacancies are easily emitted into the matrix due to the recombination between the vacancies and SIAs, which induces no pronounced increase or decrease of vacancies and SIAs in the matrix, leading to no remarkable impact on the I-loop nucleation. On the other hand, the bubble formation depends much on the existence of helium, in which the number density of bubbles for PHe = 10-7 and 10-5 appm He/s is much higher than that for PHe = 0. This is because helium atoms trapped in a bubble increase the vacancy binding energy, and suppress the vacancy dissociation from the bubble, resulting in a promotion of the bubble nucleation. And then, the helium effect on the promotion of bubble nucleation is very strong, even the number of helium atoms in a bubble is not so large.

  5. The Chemistry of the Noble Gases, Understanding the Atom Series.

    Science.gov (United States)

    Chernick, Cedric L.

    The history of the discovery, isolation, characterization, production and use of argon, krypton, xenon, helium, and radon is followed by an account of early attempts to react them with other elements. The use of the electron shell theory of valence to explain their inertness and the reactions of chemists to the production of xenon compounds is…

  6. Formation of K*He Exciplexes on the Surface of Helium Nanodroplets Studied in Real Time

    Science.gov (United States)

    Schulz, C. P.; Claas, P.; Stienkemeier, F.

    2001-10-01

    Superfluid helium nanodroplets are doped with potassium atoms to form complexes with the alkali atom residing on the surface of the droplets. Dispersed laser-induced fluorescence spectra of such systems already revealed the formation of M*He ( M = Na,K) exciplexes upon electronic excitation [Reho et al., Faraday Discuss. 108, 161 (1997)]. By means of femtosecond pump-probe spectroscopy, this formation process now is followed in real time. We find K*Hen = 1 to be formed within 180 fs. Furthermore, the existence of exciplexes with n>1 is quantified suggesting that the first ring around the potassium atom contains four helium atoms.

  7. Helium in Earth's early core

    Science.gov (United States)

    Bouhifd, M. A.; Jephcoat, Andrew P.; Heber, Veronika S.; Kelley, Simon P.

    2013-11-01

    The observed escape of the primordial helium isotope, 3He, from the Earth's interior indicates that primordial helium survived the energetic process of planetary accretion and has been trapped within the Earth to the present day. Two distinct reservoirs in the Earth's interior have been invoked to account for variations in the 3He/4He ratio observed at the surface in ocean basalts: a conventional depleted mantle source and a deep, still enigmatic, source that must have been isolated from processing throughout Earth history. The Earth's iron-based core has not been considered a potential helium source because partitioning of helium into metal liquid has been assumed to be negligible. Here we determine helium partitioning in experiments between molten silicates and iron-rich metal liquids at conditions up to 16GPa and 3,000K. Analyses of the samples by ultraviolet laser ablation mass spectrometry yield metal-silicate helium partition coefficients that range between 4.7×10-3 and 1.7×10-2 and suggest that significant quantities of helium may reside in the core. Based on estimated concentrations of primordial helium, we conclude that the early core could have incorporated enough helium to supply deep-rooted plumes enriched in 3He throughout the age of the Earth.

  8. Helium and Neon in Comets

    Science.gov (United States)

    Jewitt, David

    1996-01-01

    Two comets were observed with EUVE in late 1994. Both comet Mueller and comet Borrelly are short-period comets having well established orbital elements and accurate ephemerides. Spectra of 40 ksec were taken of each. No evidence for emission lines from either Helium or Neon was detected. We calculated limits on the production rates of these atoms (relative to solar) assuming a standard isotropic outflow model, with a gas streaming speed of 1 km/s. The 3-sigma (99.7% confidence) limits (1/100,000 for He, 0.8 for Ne) are based on a conservative estimate of the noise in the EUVE spectra. They are also weakly dependent on the precise pointing and tracking of the EUVE field of view relative to the comet during the integrations. These limits are consistent with ice formation temperatures T greater than or equal to 30 K, as judged from the gas trapping experiments of Bar-Nun. For comparison, the solar abundances of these elements are He/O = 110, Ne/O = 1/16. Neither limit was as constraining as we had initially hoped, mainly because comets Mueller and Borrelly were intrinsically less active than anticipated.

  9. Quantum electrodynamics tests and X-rays standards using pionic atoms and highly charged ions; Tests d'electrodynamique quantique et etalons de rayons-X a l'aide des atomes pioniques et des ions multicharges

    Energy Technology Data Exchange (ETDEWEB)

    Martino, Trassinelli

    2005-12-15

    The object of this thesis is to present a new measurement of the pion mass using pionic nitrogen X-ray spectroscopy and results on helium-like argon and sulphur spectroscopy. The new pion mass has been measured with an accuracy of 1.7 ppm, 30% better that the present world average value, and it is obtained from Bragg spectroscopy of 5 ->4 pionic nitrogen transitions using the theoretical predictions provided by quantum electrodynamics. We have got: m({pi}{sup -}) = (139.571042 {+-} 0.000210 {+-} 0.000110) where the first error is due to the statistics and the second is the systematic error. I present the calculation of the hyperfine structure and recoil corrections for pionic atoms using a new perturbation method for the Klein-Gordon equation. The spectrometer used for this measurement has been characterized with the relativistic M1 transitions from helium-like ions produced with a new device, the Electron-Cyclotron-Resonance Ion Trap. High statistics spectra from these ions have enabled us to measure transition energies with an accuracy of some ppm which has allowed us to compare theoretical predictions with experiment data. X-ray emission from pionic atoms and multicharged ions can be used to define new types of X-ray standards for energies of a few keV.

  10. LRO-LAMP Observations of Lunar Exospheric Helium

    Science.gov (United States)

    Grava, Cesare; Retherford, Kurt D.; Hurley, Dana M.; Feldman, Paul D.; Gladstone, Randy; Greathouse, Thomas K.; Cook, Jason C.; Stern, Alan; Pryor, Wayne R.; Halekas, Jasper S.; Kaufmann, David E.

    2015-11-01

    We present results from Lunar Reconnaissance Orbiter’s (LRO) UV spectrograph LAMP (Lyman-Alpha Mapping Project) campaign to study the lunar atmosphere. Two kinds of off-nadir maneuvers (lateral rolls and pitches towards and opposite the direction of motion of LRO) were performed to search for resonantly scattering species, increasing the illuminated line-of-sight (and hence the signal from atoms resonantly scattering the solar photons) compared to previously reported LAMP “twilight observations” [Cook & Stern, 2014]. Helium was the only element distinguishable on a daily basis, and we present latitudinal profiles of its line-of-sight column density in December 2013. We compared the helium line-of-sight column densities with solar wind alpha particle fluxes measured from the ARTEMIS (Acceleration, Reconnection, Turbulence, & Electrodynamics of Moon’s Interaction with the Sun) twin spacecraft. Our data show a correlation with the solar wind alpha particle flux, confirming that the solar wind is the main source of the lunar helium, but not with a 1:1 relationship. Assuming that the lunar soil is saturated with helium atoms, our results suggest that not all of the incident alpha particles are converted to thermalized helium, allowing for a non-negligible fraction (~50 %) to escape as suprathermal helium or simply backscattered from the lunar surface. We also support the finding by Benna et al. [2015] and Hurley et al. [2015], that a non-zero contribution from endogenic helium, coming from radioactive decay of 232Th and 238U within the mantle, is present, and is estimated to be (4.5±1.2) x 106 He atoms cm-2 s-1. Finally, we compare LAMP-derived helium surface density with the one recorded by the mass spectrometer LACE (Lunar Atmospheric Composition Experiment) deployed on the lunar surface during the Apollo 17 mission, finding good agreement between the two measurements. These LRO off-nadir maneuvers allow LAMP to provide unique coverage of local solar time and

  11. Theoretical model of the helium zone plate microscope

    Science.gov (United States)

    Salvador Palau, Adrià; Bracco, Gianangelo; Holst, Bodil

    2017-01-01

    Neutral helium microscopy is a new technique currently under development. Its advantages are the low energy, charge neutrality, and inertness of the helium atoms, a potential large depth of field, and the fact that at thermal energies the helium atoms do not penetrate into any solid material. This opens the possibility, among others, for the creation of an instrument that can measure surface topology on the nanoscale, even on surfaces with high aspect ratios. One of the most promising designs for helium microscopy is the zone plate microscope. It consists of a supersonic expansion helium beam collimated by an aperture (skimmer) focused by a Fresnel zone plate onto a sample. The resolution is determined by the focal spot size, which depends on the size of the skimmer, the optics of the system, and the velocity spread of the beam through the chromatic aberrations of the zone plate. An important factor for the optics of the zone plate is the width of the outermost zone, corresponding to the smallest opening in the zone plate. The width of the outermost zone is fabrication limited to around 10 nm with present-day state-of-the-art technology. Due to the high ionization potential of neutral helium atoms, it is difficult to build efficient helium detectors. Therefore, it is crucial to optimize the microscope design to maximize the intensity for a given resolution and width of the outermost zone. Here we present an optimization model for the helium zone plate microscope. Assuming constant resolution and width of the outermost zone, we are able to reduce the problem to a two-variable problem (zone plate radius and object distance) and we show that for a given beam temperature and pressure, there is always a single intensity maximum. We compare our model with the highest-resolution zone plate focusing images published and show that the intensity can be increased seven times. Reducing the width of the outermost zone to 10 nm leads to an increase in intensity of more than 8000

  12. Search for WIMPs in liquid argon

    CERN Document Server

    Amsler, C

    2011-01-01

    Our group from the University of Zurich is performing R&D work towards the design of a large liquid argon detector to detect Weakly Interacting Massive Particles (WIMPs). This project is developed within the DARWIN Collaboration funded by ASPERA to prepare a proposal for the next generation of WIMP searches using noble liquids. We are performing R&D to detect the VUV light from recoiling argon nuclei. Results obtained with one ton of liquid argon (ArDM prototype) and prospects using a monoenergetic neutron source are discussed.

  13. Helium production cross section Measurement of Pb and Sn for 14.9 MeV neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Takao, Yoshiyuki; Fujimoto, Toshihiro; Ozaki, Shuji; Muramasu, Masatomo; Nakashima, Hideki [Kyushu Univ., Fukuoka (Japan); Kanda, Yukinori; Ikeda, Yujiro

    1998-03-01

    Helium production cross sections of lead and tin for 14.9 MeV neutrons were measured by helium accumulation method. Lead and tin samples were irradiated with FNS, an intense d-T neutron source of JAERI. The amount of helium produced in the samples by the neutron irradiation was measured with the Helium Atoms Measurement System (HAMS) at Kyushu University. As the samples contained a small amount of helium because of their small helium production cross sections at 14.9 MeV, the samples were evaporated by radiation from a tungsten filament to decrease background gases at helium measurement. Uncertainties of the present results were less than {+-}4.4%. The results were compared with other experimental data in the literature and also compared with the evaluated values in JENDL-3.2. (author)

  14. Quantum control of the XUV photoabsorption sp ectrum of helium atoms via the carrier-envelop e-phase of an infrared laser pulse%红外激光载波包络相位对氦原子的极紫外光(XUV)吸收谱的量子调控研究∗

    Institute of Scientific and Technical Information of China (English)

    杨增强; 张力达

    2015-01-01

    In the present paper, we investigate the quantum control of the XUV photoabsorption spectrum of helium atoms via the carrier-envelope-phase (CEP) of an infrared (IR) laser pulse by numerically solving the time-dependent one-dimensional (1D) two-electron Schrödinger equation. The advantage of the 1D model is that the associated time-dependent Schrodinger equation (TDSE) can be solved numerically with high precision as taking full account of the interaction between the electrons and without making any assumptions about the dominant physical mechanisms. In our study, a single attosecond XUV pulse with broad bandwidth is used to create a wave packet consisting of several doubly-excited states. Helium atoms subjected to the XUV pulse can be ionized through two different pathways: either direct ionization into the continuum or indirect ionization via the autoionization of doubly excited states. The interference of these two paths gives rise to the well-known Fano line shape in the photoabsorption spectrum, which is determined by the ratio and relative phases of the two paths. In the presence of an IR laser pulse, however, we find that the Fano line profiles are strongly modified, in good agreement with recent experimental observations [C. Ott et al., Science 340, 716 (2013); C. Ott et al., Nature 516, 374 (2014)]. At certain time delays, we can observe symmetric Lorentz, inverted Fano profiles, and even negative absorption cross sections, indicating that the XUV light can be amplified during the interaction with atoms. We fit the absorption spectra with the Fano line profiles giving rise to the CEP-dependent Fano q parameters, which are modulated from extremely large positive value to extremely large negative value. Since the q parameter is proportional to the ratio between the dipole matrix of the indirect ionization path and the dipole matrix of the direct ionization path;these results indicate that the quantum interference between the two ionization paths can be e

  15. Influence of the bath gas on the condensation of supersaturated iron atom vapour at room temperature

    Science.gov (United States)

    Eremin, A.; Gurentsov, E.; Schulz, C.

    2008-03-01

    The influence of the kind of bath gas and its pressure on the iron nanoparticle formation and growth was investigated experimentally. Iron nanoparticles were synthesized from supersaturated iron vapour generated by ArF excimer laser pulse photolysis of gaseous Fe(CO)5 at room temperature. The particle size was determined by time-resolved laser-induced incandescence (TiRe-LII) as a function of time after photolysis at different experimental conditions. Additionally, final particles were sampled and analysed by transmission electron microscopy and by energy-dispersive x-ray analysis. The particle growth rate and the final particle size depended on the bath-gas composition and pressure. Increasing the argon bath-gas pressure accelerated the iron nanoparticle growth rate. In contrast to argon, no influence of helium on the particle growth rate was observed. The experimental results are compared with numerical simulations of particle surface growth, based on the model developed in previous investigations. The simulations indicate that the observed differences in the influence of the bath gas on the particle formation are caused by the species-dependent quenching probability of the active atom-particle complexes by the bath gas.

  16. High Efficiency Regenerative Helium Compressor Project

    Data.gov (United States)

    National Aeronautics and Space Administration — Helium plays several critical rolls in spacecraft propulsion. High pressure helium is commonly used to pressurize propellant fuel tanks. Helium cryocoolers can be...

  17. Transmission Electron Microscopy Characterization of Helium Bubbles in Aged Plutonium

    Energy Technology Data Exchange (ETDEWEB)

    Schwartz, A J; Wall, M A; Zocco, T G; Blobaum, K M

    2004-11-02

    The self-irradiation damage generated by alpha decay of plutonium results in the formation of lattice defects, helium, and uranium atoms. Over time, microstructural evolution resulting from the self-irradiation may influence the physical and mechanical properties of the material. In order to assess microstructural changes, we have developed and applied procedures for the specimen preparation, handling, and transmission electron microscopy characterization of Pu alloys. These transmission electron microscopy investigations of Pu-Ga alloys ranging in age up to 42-years old reveal the presence of nanometer-sized helium bubbles. The number density of bubbles and the average size have been determined for eight different aged materials.

  18. Radioactive core ions of microclusters, ``snowballs`` in superfluid helium

    Energy Technology Data Exchange (ETDEWEB)

    Takahashi, N. [Osaka Univ., Toyonaka (Japan). Dept. of Physics; Shimoda, T. [Osaka Univ., Toyonaka (Japan). Dept. of Physics; Fujita, Y. [Osaka Univ., Toyonaka (Japan). Dept. of Physics; Miyatake, H. [Osaka Univ., Toyonaka (Japan). Dept. of Physics; Mizoi, Y. [Osaka Univ., Toyonaka (Japan). Dept. of Physics; Kobayashi, H. [Osaka Univ., Toyonaka (Japan). Dept. of Physics; Sasaki, M. [Osaka Univ., Toyonaka (Japan). Dept. of Physics; Shirakura, T. [Osaka Univ., Toyonaka (Japan). Dept. of Physics; Itahashi, T. [Research Center for Nuclear Physics, Osaka Univ., Ibaraki (Japan); Mitsuoka, S. [Research Center for Nuclear Physics, Osaka Univ., Ibaraki (Japan); Matsukawa, T. [Naruto Univ. of Education, Tokushima (Japan); Ikeda, N. [Kyushu Univ., Fukuoka (Japan). Dept. of Physics; Morinobu, S. [Kyushu Univ., Fukuoka (Japan). Dept. of Physics; Hinde, D.J. [Australian National Univ., Canberra, ACT (Australia). Research School of Physical Sciences; Asahi, K. [Tokyo Inst. of Tech. (Japan). Dept. of Physics; Ueno, H. [Tokyo Inst. of Tech. (Japan). Dept. of Physics; Izumi, H. [Tokyo Inst. of Tech. (Japan). Dept. of Physics

    1996-12-01

    Short-lived beta-ray emitters, {sup 12}B, sustaining nuclear spin polarization were introduced into superfluid helium. The nuclear polarization of {sup 12}B was observed via measurement of beta-ray asymmetry. It was found that the nuclear polarization was preserved throughout the lifetime of {sup 12}B (20.3 ms). This suggests that the ``snowball``, an aggregation of helium atoms produced around an alien ion, constitutes a suitable milieu for freezing-out the nuclear spin of the core ion and that most likely the solidification takes place at the interior of the aggregation. (orig.).

  19. Cavitation in liquid helium

    Energy Technology Data Exchange (ETDEWEB)

    Finch, R. D.; Kagiwada, R.; Barmatz, M.; Rudnick, I.

    1963-11-15

    Ultrasonic cavitation was induced in liquid helium over the temperature range 1.2 to 2.3 deg K, using a pair of identical transducers. The transducers were calibrated using a reciprocity technique and the cavitation threshold was determined at 90 kc/s. It was found that this threshold has a sharp peak at the lambda point, but is, at all temperatures quite low, with an approximate range of 0.001 to 0.01 atm. The significance of the results is discussed. (auth)

  20. Analysis of Photoassociation Spectra for Giant Helium Dimers

    CERN Document Server

    Léonard, J; Walhout, M; Van der Straten, P; Leduc, M

    2004-01-01

    We perform a theoretical analysis to interpret the spectra of purely long-range helium dimers produced by photoassociation (PA) in an ultra-cold gas of metastable helium atoms. The experimental spectrum obtained with the PA laser tuned closed to the $2^3S_1\\leftrightarrow 2^3P_0$ atomic line has been reported in a previous Letter. Here, we first focus on the corrections to be applied to the measured resonance frequencies in order to infer the molecular binding energies. We then present a calculation of the vibrational spectra for the purely long-range molecular states, using adiabatic potentials obtained from perturbation theory. With retardation effects taken into account, the agreement between experimental and theoretical determinations of the spectrum for the $0_u^+$ purely long-range potential well is very good. The results yield a determination of the lifetime of the $2^3P$ atomic state.

  1. Clinical periodontics with the argon laser

    Science.gov (United States)

    Finkbeiner, R. L.

    1995-04-01

    The argon laser has proven to be a valuable tool for the thermodynamic debridement of the periodontal lesion, incisions and tissue fusion. Illustrations of clinical applications and discussion of laser parameters will be provided.

  2. New level-resolved collision data for neutral argon, benchmarked against the ALEXIS plasma experiment

    Science.gov (United States)

    Arnold, Nicholas; Loch, Stuart; Ballance, Connor; Thomas, Ed

    2016-10-01

    Performing spectroscopic measurements of emission lines in low temperature laboratory plasmas is challenging because the plasma is often neutral-dominated and not in thermal equilibrium. The densities and temperatures are such that coronal models do not apply; meaning that generalized collisional-radiative (GCR) methods must be employed to theoretically analyze atomic processes. However, for most noble gases, detailed, level-resolved atomic data for neutral and low-charge states does not exist in the literature. We report on a new project, where we use existing atomic physics codes to calculate level-resolved atomic data for neutral and low charge states of argon and compare with previously published, term-resolved theoretical results. In addition, we use the Atomic Structure and Data Analysis (ADAS) suite of codes to calculate a GCR model for low temperature neutral argon, which we compare to published measurements of argon optical emission cross sections. Finally, we compare synthetic spectra generated from our data with observations taken from the Auburn Linear Experiment for Instability Studies (ALEXIS) in an attempt to develop new optical plasma diagnostics for electron temperature and plasma density measurements. This project is supported by the U.S. Department of Energy. Grant Number: DE-FG02-00ER54476.

  3. Melting of "non-magic" argon clusters and extrapolation to the bulk limit

    Science.gov (United States)

    Senn, Florian; Wiebke, Jonas; Schumann, Ole; Gohr, Sebastian; Schwerdtfeger, Peter; Pahl, Elke

    2014-01-01

    The melting of argon clusters ArN is investigated by applying a parallel-tempering Monte Carlo algorithm for all cluster sizes in the range from 55 to 309 atoms. Extrapolation to the bulk gives a melting temperature of 85.9 K in good agreement with the previous value of 88.9 K using only Mackay icosahedral clusters for the extrapolation [E. Pahl, F. Calvo, L. Koči, and P. Schwerdtfeger, "Accurate melting temperatures for neon and argon from ab initio Monte Carlo simulations," Angew. Chem., Int. Ed. 47, 8207 (2008)]. Our results for argon demonstrate that for the extrapolation to the bulk one does not have to restrict to magic number cluster sizes in order to obtain good estimates for the bulk melting temperature. However, the extrapolation to the bulk remains a problem, especially for the systematic selection of suitable cluster sizes.

  4. Atomistic-Continuum Hybrid Simulation of Heat Transfer between Argon Flow and Copper Plates

    CERN Document Server

    Mao, Yijin; Chen, C L

    2016-01-01

    A simulation work aiming to study heat transfer coefficient between argon fluid flow and copper plate is carried out based on atomistic-continuum hybrid method. Navier-Stokes equations for continuum domain are solved through the Pressure Implicit with Splitting of Operators (PISO) algorithm, and the atom evolution in molecular domain is solved through the Verlet algorithm. The solver is validated by solving Couette flow and heat conduction problems. With both momentum and energy coupling method applied, simulations on convection of argon flows between two parallel plates are performed. The top plate is kept as a constant velocity and has higher temperature, while the lower one, which is modeled with FCC copper lattices, is also fixed but has lower temperature. It is found that, heat transfer between argon fluid flow and copper plate in this situation is much higher than that at macroscopic when the flow is fully developed.

  5. Regimes Of Helium Burning

    CERN Document Server

    Timmes, F X

    2000-01-01

    The burning regimes encountered by laminar deflagrations and ZND detonations propagating through helium-rich compositions in the presence of buoyancy-driven turbulence are analyzed. Particular attention is given to models of X-ray bursts which start with a thermonuclear runaway on the surface of a neutron star, and the thin shell helium instability of intermediate-mass stars. In the X-ray burst case, turbulent deflagrations propagating in the lateral or radial directions encounter a transition from the distributed regime to the flamlet regime at a density of 10^8 g cm^{-3}. In the radial direction, the purely laminar deflagration width is larger than the pressure scale height for densities smaller than 10^6 g cm^{-3}. Self-sustained laminar deflagrations travelling in the radial direction cannot exist below this density. Similarily, the planar ZND detonation width becomes larger than the pressure scale height at 10^7 g cm^{-3}, suggesting that a steady-state, self-sustained detonations cannot come into exista...

  6. Argon Laser Photoablation for Postburn Conjunctival Pigmentation

    Directory of Open Access Journals (Sweden)

    Seong Joon Ahn

    2014-01-01

    Full Text Available We report a case of an ocular burn injury from boiling water which resulted in conjunctival pigmentation, 1 week following injury. For cosmetic purposes, 2 sessions of argon laser photoablation were performed. One month after laser treatment, conjunctival pigmentation had been successfully removed and the patient was very satisfied with the results. Argon laser photoablation may be an effective way to remove postburn conjunctival pigmentation.

  7. Helium diffusion in carbonates

    Science.gov (United States)

    Amidon, W. H.; Cherniak, D. J.; Watson, E. B.; Hobbs, D.

    2013-12-01

    The abundance and large grain size of carbonate minerals make them a potentially attractive target for 4He thermochronology and 3He cosmogenic dating, although the diffusive properties of helium in carbonates remain poorly understood. This work characterizes helium diffusion in calcite and dolomite to better understand the crystal-chemical factors controlling He transport and retentivity. Slabs of cleaved natural calcite and dolomite, and polished sections of calcite cut parallel or normal to c, were implanted with 3He at 3 MeV with a dose of 5x1015/cm2. Implanted carbonates were heated in 1-atm furnaces, and 3He distributions following diffusion anneals were profiled with Nuclear Reaction Analysis using the reaction 3He(d,p)4He. For 3He transport normal to cleavage surfaces in calcite, we obtain the following Arrhenius relation over the temperature range 78-300°C: Dcalcite = 9.0x10-9exp(-55 × 6 kJ mol-1/RT) m2sec-1. Diffusion in calcite exhibits marked anisotropy, with diffusion parallel to c about two orders of magnitude slower than diffusion normal to cleavage faces. He diffusivities for transport normal to the c-axis are similar in value to those normal to cleavage surfaces. Our findings are broadly consistent with helium diffusivities from step-heating measurements of calcite by Copeland et al. (2007); these bulk degassing data may reflect varying effects of diffusional anisotropy. Helium diffusion normal to cleavage surfaces in dolomite is significantly slower than diffusion in calcite, and has a much higher activation energy for diffusion. For dolomite, we obtain the following Arrhenius relation for He diffusion over the temperature range 150-400°C: Ddolomite = 9.0x10-8exp(-92 × 9 kJ mol-1/RT) m2sec-1. The role of crystallographic structure in influencing these differences among diffusivities was evaluated using the maximum aperture approach of Cherniak and Watson (2011), in which crystallographic structures are sectioned along possible diffusion

  8. Helium in near Earth orbit

    CERN Document Server

    Alcaraz, J; Ambrosi, G; Anderhub, H; Ao, L; Arefev, A; Azzarello, P; Babucci, E; Baldini, L; Basile, M; Barancourt, D; Barão, F; Barbier, G; Barreira, G; Battiston, R; Becker, R; Becker, U; Bellagamba, L; Béné, P; Berdugo, J; Berges, P; Bertucci, B; Biland, A; Bizzaglia, S; Blasko, S; Bölla, G; Boschini, M; Bourquin, Maurice; Brocco, L; Bruni, G; Buénerd, M; Burger, J D; Burger, W J; Cai, X D; Camps, C; Cannarsa, P; Capell, M; Casadei, D; Casaus, J; Castellini, G; Cecchi, C; Chang, Y H; Chen, H F; Chen, H S; Chen, Z G; Chernoplekov, N A; Tzi Hong Chiueh; Chuang, Y L; Cindolo, F; Commichau, V; Contin, A; Cristinziani, M; Da Cunha, J P; Dai, T S; Deus, J D; Dinu, N; Djambazov, L; D'Antone, I; Dong, Z R; Emonet, P; Engelberg, J; Eppling, F J; Eronen, T; Esposito, G; Extermann, Pierre; Favier, Jean; Fiandrini, E; Fisher, P H; Flügge, G; Fouque, N; Galaktionov, Yu; Gervasi, M; Giusti, P; Grandi, D; Grimm, O; Gu, W Q; Hangarter, K; Hasan, A; Hermel, V; Hofer, H; Huang, M A; Hungerford, W; Ionica, M; Ionica, R; Jongmanns, M; Karlamaa, K; Karpinski, W; Kenney, G; Kenny, J; Kim, W; Klimentov, A; Kossakowski, R; Koutsenko, V F; Kräber, M H; Laborie, G; Laitinen, T; Lamanna, G; Laurenti, G; Lebedev, A; Lee, S C; Levi, G; Levchenko, P M; Liu, C L; Liu Hong Tao; Lopes, I; Lu, G; Lü, Y S; Lübelsmeyer, K; Luckey, D; Lustermann, W; Maña, C; Margotti, A; Mayet, F; McNeil, R R; Meillon, B; Menichelli, M; Mihul, A; Mourão, A M; Mujunen, A; Palmonari, F; Papi, A; Park, I H; Pauluzzi, M; Pauss, Felicitas; Perrin, E; Pesci, A; Pevsner, A; Pimenta, M; Plyaskin, V; Pozhidaev, V; Pohl, M; Postolache, V; Produit, N; Rancoita, P G; Rapin, D; Raupach, F; Ren, D; Ren, Z; Ribordy, M; Richeux, J P; Riihonen, E; Ritakari, J; Röser, U; Roissin, C; Sagdeev, R; Sartorelli, G; Schultz von Dratzig, A; Schwering, G; Scolieri, G; Seo, E S; Shoutko, V; Shoumilov, E; Siedling, R; Son, D; Song, T; Steuer, M; Sun, G S; Suter, H; Tang, X W; Ting, Samuel C C; Ting, S M; Tornikoski, M; Torsti, J; Trümper, J E; Ulbricht, J; Urpo, S; Usoskin, I; Valtonen, E; Van den Hirtz, J; Velcea, F; Velikhov, E P; Verlaat, B; Vetlitskii, I; Vezzu, F; Vialle, J P; Viertel, Gert M; Vitè, Davide F; Von Gunten, H P; Waldmeier-Wicki, S; Wallraff, W; Wang, B C; Wang, J Z; Wang, Y H; Wiik, K; Williams, C; Wu, S X; Xia, P C; Yan, J L; Yan Lu Guang; Yang, C G; Yang, M; Ye Shu Wei; Yeh, P; Xu, Z Z; Zhang, H Y; Zhang, Z P; Zhao, D X; Zhu, G Y; Zhu, W Z; Zhuang, H L; Zichichi, A; Zimmermann, B; Zuccon, P

    2000-01-01

    The helium spectrum from 0.1 to 100 GeV/nucleon was measured by the Alpha Magnetic Spectrometer (AMS) during space shuttle flight STS-91 at altitudes near 380 km. Above the geomagnetic cutoff the spectrum is parameterized by a power law. Below the geomagnetic cutoff a second helium spectrum was observed. In the second helium spectra over the energy range 0.1 to 1.2 GeV/nucleon the flux was measured to be (6.3+or-0.9)*10/sup -3/ (m/sup 2/ sec sr)/sup -1/ and more than ninety percent of the helium was determined to be /sup 3/He (at the 90% CL). Tracing helium from the second spectrum shows that about half of the /sup 3/He travel for an extended period of time in the geomagnetic field and that they originate from restricted geographic regions similar to protons and positrons. (22 refs).

  9. Effects of helium on titanium films and the helium diffusion

    Institute of Scientific and Technical Information of China (English)

    SONG YingMin; LUO ShunZhong; LONG XingGui; AN Zhu; LIU Ning; PANG HongChao; WU XingChun; YANG BenFu; ZHENG SiXiao

    2008-01-01

    Using direct current-magnetron sputtering, Helium-trapped Ti films with a He/Ar mixture was studied. The relative helium content, helium depth profiles for the Ti films and crystallization capacity were analyzed by Enhanced Proton Backscattering Spectrometry (EPBS) and X-ray diffraction (XRD). It was found that helium diffusion enhanced as more helium trapping into Ti films, and the He holding ratios were 95.9%, 94.9%, 93.9%, 82.8% when the Ti films with the He/Ti of concentrations of 9.7 at.Q, 19.5 at.Q, 19.7 at.Q, 48.3 at.% were measured again 4 months later, respectively. The diffraction peaks be-came weak and wider, the peak of (002) plane was shifted to smaller diffraction angles and the relevant interplanar spacing d(hkl) increased gradually as more helium trapping into Ti films. The main peak was made trending to the (101) plane by both higher deposition temperature and more helium trapping.

  10. Potassium-argon/argon-40-argon-39 geochronology of Cenozoic alkali basalts from the South China Sea

    Institute of Scientific and Technical Information of China (English)

    YAN Quanshu; SHI Xuefa; YANG Yaomin; WANG Kunshan

    2008-01-01

    Based on the isotopic chronologic results of Cenozoic alkali basalts from the South China Sea,the characteristics of volcanic activi-ty of the South China Sea after spreading were studied.The potassium - argon ages of eight alkali basalt samples from the South China Sea,and the argon - argon ages of two samples among them are reported.Apparent ages of the whole rock are 3.80 to 7.91 Ma with an average value of 5.43 Ma (potassium- argon,whole rock),and there is little difference among samples at the same location,e.g.,4.76~5.78 Ma for location S04-12.The argon - argon ages for the two samples are 6.06 and 4.71 Ma,which lie within the age scope of potassium - argon method.The dating results indicate that rock-forming age is from late Miocene to Pli-ocene,which is consistent with erupting event for alkali basalts from adjacent regions of the South China Sea.Volcanic activities occur after the cessation of spreading of the South China Sea,which are controlled by lithospheric fault and the spreading center formed during the spreading period of the South China Sea.These dating results,combined with geochemical characteristics of these basalts,the published chronological data for the South China Sea and its adjacent regions,and the updated geophysical data near Hainan Island,suggest that after the cessation of spreading of the South China Sea,there occur widely distributing magmatic activities which primarily is alkali basalt,and the volcanic activity continues to Quaternary.The activity may be relative to Hainan mantle plume originated from core/mantle boundary.

  11. Phonon amplification using evaporation and adsorption of helium

    Energy Technology Data Exchange (ETDEWEB)

    More, T.; Adams, J.S.; Bandler, S.R.; Broueer, S.M.; Lanou, R.E.; Maris, H.J.; Seidel, G.M. [Department of Physics, Brown University, Providence, Rhode Island 02912 (United States)

    1996-07-01

    We report the results of experiments designed to investigate the feasibility of amplifying a phonon signal using the evaporation of helium from a superfluid film and its subsequent readsorption onto a helium-free surface. We envision a multistage amplifier in which helium is evaporated from a wafer with a helium film only on one side and then adsorbed onto the film-free surface of a similar wafer. The phonons created by the adsorption reach the film on the opposite side of the wafer and potentially desorb more helium than was evaporated by the first wafer. The amplification would come from the high ratio of the binding energy of a helium atom to a film-free surface relative to the binding energy to the liquid. A number of experiments are reported that investigate the efficiencies of the individual steps of the process. The gain per stage is found to be about 3 for high-energy densities in which multiphonon processes are possible. At low-energy densities, the energy deposited into a film-free wafer is found to be less than the original input energy, with the ratio of output to input energy 0.2. Since in applications requiring amplification the phonon density produced by the adsorption of helium on a wafer will be low, the configuration we have studied{emdash}phonons produced in silicon coated with a saturated {sup 4}He film{emdash}will not result in amplification. However, other configurations might improve the efficiency enough to make an amplifier possible. {copyright} {ital 1996 The American Physical Society.}

  12. Luminescence studies of trace gases through metastable transfer in cold helium jets

    Science.gov (United States)

    Wilde, Scott Colton

    Among the elements, Helium has the largest steps among its internal energy structure that can keep for long periods of time, hence the metastable helium moniker. It is referred to as a "nano-grenade" in some circles because of how much energy it can deliver to a space roughly the size of an atom. This work demonstrates a method to create metastable helium abundantly and it is used to excite trace amounts of oxygen to the point where the signal received from the oxygen was larger than the signal received from the helium in a cold atomized jet. Further cooling of the jet and turbulence added by a liquid helium surface worked to increase the oxygen signal and decrease the helium signal. This work investigates the possibility of forming a strong metastable helium source from a flowing helium gas jet excited by passing through ring electrodes introduced into a cryogenic environment using evaporated helium as a buffer gas. Prior study of luminescence from trace gases at cold helium temperatures is virtually absent and so it is the motivation for this work to blaze the trail in this subject. The absence of ionic oxygen spectral lines from the transfer of energy that was well over the first ionization potential of oxygen made for a deeper understanding of collision dynamics with multiple collision partners. This opened the possibility of using the high energy states of oxygen after metastable transfer as a lasing transition previously unavailable and a preliminary analysis suggested that the threshold for lasing action should be easily overcome if feedback were introduced by an optical cavity. To better understand the thermodynamics of the jet it was proposed to use diatomic nitrogen as an in situ thermometer, investigating whether the rotational degrees of freedom of the nitrogen molecule were in thermal equilibrium with the surrounding environment. If the gas was truly in thermodynamic equilibrium then the temperature given by the method of using collisions of a buffer

  13. Stability of helium bubbles in alpha-iron: A molecular dynamics study

    Energy Technology Data Exchange (ETDEWEB)

    Lucas, G. [Ecole Polytechnique Federale de Lausanne (EPFL), Centre de Recherche en Physique des Plasmas, Association Euratom-Confederation Suisse, CH 5332 Villigen PSI (Switzerland)], E-mail: guillaume.lucas@psi.ch; Schaeublin, R. [Ecole Polytechnique Federale de Lausanne (EPFL), Centre de Recherche en Physique des Plasmas, Association Euratom-Confederation Suisse, CH 5332 Villigen PSI (Switzerland)

    2009-04-30

    Molecular dynamics simulations were performed to estimate the dissociation energies of helium interstitials, vacancies and self-interstitial atoms from small helium-vacancy clusters. Several sets of empirical potentials have been tested and compared with available ab initio calculations in order to provide the best combination of potentials to study the stability of small helium bubbles. The behavior of the cluster seems to be better described using Ackland potential for the Fe-Fe interactions and Juslin potential for the Fe-He interactions. From the calculations, it appears that the dissociation energies mainly depend on the helium-to-vacancy ratio rather than the cluster size. The helium/vacancy crossover slightly varies with increasing number of vacancies, but the crossover defining the loop-punching regime decreases strongly with increasing cluster sizes.

  14. Radiation damage in gallium-stabilized δ-plutonium with helium bubbles

    Science.gov (United States)

    Wu, FengChao; Wang, Pei; Liu, XiaoYi; Wu, HengAn

    2017-02-01

    To understand the role of helium on self-irradiation effects in δ-plutonium, microstructure evolutions due to α-decay events near pre-existing helium bubbles in gallium-stabilized δ-plutonium are investigated using molecular dynamics simulations. Bubble promoting effect plays a dominating role in point defects production, resulting in increasing number of point defects. When lightweight helium atoms act as media, energy transfer discrepancy and altered spatial morphology of point defects induced by mass effect are revealed. The evolution of stacking faults surrounding the disordered core is studied and their binding effect on the propagation of point defects are presented. The cascade-induced bubble coalescence, resolution and re-nucleation driven by internal pressure are obtained in the investigation on helium behaviors. The intrinsic tendency in our simulated self-irradiation with helium bubbles is significant for understanding the underlying mechanism of aging in plutonium and its alloys.

  15. High Pressure Equation of State Studies Using Ethanol-Methanol And Argon As Pressure Medium

    Science.gov (United States)

    Godwal, B. K.; Speziale, S.; Clark, S.; Yan, J.; Jeanloz, R.

    2008-12-01

    Experimental high pressure studies are extremely important to planetary science, material science and to the development of condensed matter theory. With experimental difficulties in creating the extreme pressure temperature conditions appropriate to planetary interiors, the approach used is to obtain the thermodynamic data on materials of interest by extrapolating the condensed matter theory which has been benchmarked with the outcome of high pressure experiments to the available high pressures. However the high pressure data used to match the theory heavily depends on the use of pressure media; like ethanol-methanol, silicon oil, argon and helium. Unfortunately still there exist controversy in the literature even with the use of helium as pressure medium as illustrated by the unsettled debate on Zn and Os among different groups. We have measured the equation of state of intermetallic compound AuIn2 and Cd0.8Hg0.2 alloy using ethanol-methanol and argon to the pressure of 20 GPa to confirm the appearance of anomalies in the data due to occurrence of subtle electronic phase transitions. However these anomalies can also be attributed to oriented lattice strains and local non-hydrostatic conditions. We have tried to remove these at room temperature by stabilizing the sample in argon medium in the diamond anvil cell with proper annealing as indicated by the uniformity of the pressure across the sample by ruby fluorescence measurements. We will present the data revealing the electronic transition in AuIn2 at 2.7 GPa and in Cd0.8Hg0.2 near 9 and 18 GPa.

  16. CFD Analysis on the Passive Heat Removal by Helium and Air in the Canister of Spent Fuel Dry Storage System

    Energy Technology Data Exchange (ETDEWEB)

    Shin, Do Young; Jeong, Ui Ju; Kim, Sung Joong [Hanyang University, Seoul (Korea, Republic of)

    2016-05-15

    In the current commercial design, the canister of the dry storage system is mainly backfilled with helium gas. Helium gas shows very conductive behavior due to high thermal conductivity and small density change with temperature. However, other gases such as air, argon, or nitrogen are expected to show effective convective behavior. Thus these are also considered as candidates for the backfill gas to provide effective coolability. In this study, to compare the dominant cooling mechanism and effectiveness of cooling between helium gas and air, a computational fluid dynamics (CFD) analysis for the canister of spent fuel dry storage system with backfill gas of helium and air is carried out. In this study, CFD simulations for the helium and air backfilled gas for dry storage system canister were carried out using ANSYS FLUENT code. For the comparison work, two backfilled fluids were modeled with same initial and boundary conditions. The observed major difference can be summarized as follows. - The simulation results showed the difference in dominant heat removal mechanism. Conduction for helium, and convection for air considering Reynolds number distribution. - The temperature gradient inside the fuel assembly showed that in case of air, more effective heat mixing occurred compared to helium.

  17. Thermohydraulics of a horizontal diphasic flow of superfluid helium; Thermo-hydraulique d'un ecoulement horizontal d'helium superfluide diphasique

    Energy Technology Data Exchange (ETDEWEB)

    Perraud, S

    2007-12-15

    This study aims at characterizing helium two phase flows, and to identify the dependence of their characteristics on various thermo-hydraulic parameters: vapour velocity, liquid height, vapour density, specificities of superfluidity. Both the engineer and the physicist's points of view are taken into consideration: the first one in terms of optimization of a particular cooling scheme based on a two-phase flow, and these second one in terms of more fundamental atomization-related questions. It has been shown that for velocities around 3 to 4 m/s, the liquid phase that was initially stratified undergoes an atomization through the presence of a drop haze carried by the vapor phase.This happens for superfluid helium as well as for normal helium without main differences on atomization.

  18. Electronic properties of physisorbed helium

    Energy Technology Data Exchange (ETDEWEB)

    Kossler, Sarah

    2011-09-22

    This thesis deals with electronic excitations of helium physisorbed on metal substrates. It is studied to what extent the electronic properties change compared to the gas phase due to the increased helium density and the proximity of the metal. Furthermore, the influence of different substrate materials is investigated systematically. To this end, up to two helium layers were adsorbed onto Ru (001), Pt (111), Cu (111), and Ag (111) surfaces in a custom-made cryostat. These samples were studied spectroscopically using synchrotron radiation and a time-of-flight detector. The experimental results were then analyzed in comparison with extensive theoretical model calculations.

  19. Transferring superfluid helium in space

    Science.gov (United States)

    Kittel, Peter

    1986-01-01

    A simple thermodynamic model of a transfer system for resupplying liquid helium in space is presented, with application to NASA projects including the Space Infrared Telescope Facility, the Large Deployable Reflector, and the Hubble Space Telescope. The relations between different thermodynamic regimes that can be expected in the transfer line are used to study the relative efficiencies of various possible transfer techniques. Low heat leak into the transfer line, particularly at point sources such as the coupling, is necesssary for efficient transfer of liquid helium, and proper selection of supply tank temperature is important during helium resupply.

  20. Resistor monitors transfer of liquid helium

    Science.gov (United States)

    Hesketh, W. D.

    1966-01-01

    Large resistance change of a carbon resistor at the liquid helium temperature distinguishes between the transfer of liquid helium and gaseous helium into a closed Dewar. The resistor should be physically as small as possible to reduce the heat load to the helium.

  1. Solvation of Na+, K+, and their dimers in helium.

    Science.gov (United States)

    An der Lan, Lukas; Bartl, Peter; Leidlmair, Christian; Jochum, Roland; Denifl, Stephan; Echt, Olof; Scheier, Paul

    2012-04-02

    Helium atoms bind strongly to alkali cations which, when embedded in liquid helium, form so-called snowballs. Calculations suggest that helium atoms in the first solvation layer of these snowballs form rigid structures and that their number (n) is well defined, especially for the lighter alkalis. However, experiments have so far failed to accurately determine values of n. We present high-resolution mass spectra of Na(+)He(n), K(+)He(n), Na(2)(+)He(n) and K(2)(+)He(n), formed by electron ionization of doped helium droplets; the data allow for a critical comparison with several theoretical studies. For sodium and potassium monomers the spectra indicate that the value of n is slightly smaller than calculated. Na(2)(+)He(n) displays two distinct anomalies at n=2 and n=6, in agreement with theory; dissociation energies derived from experiment closely track theoretical values. K(2)(+)He(n) distributions are fairly featureless, which also agrees with predictions.

  2. Analysis of the time-domain spectrum of hydrogen in electric field near helium surface

    Institute of Scientific and Technical Information of China (English)

    Xiaoqing Gong; Guangcan Yang

    2011-01-01

    The Ryderberg electronic wave packet dynamics of hydrogen atom near helium surface in an electric field is investigated using the semiclassical method. The autocorrelation function is calculated when the photoionized electron is excited by a short laser pulse for different atom-surface separations. The results show that new recurrences appear because of the helium surface, and the number of recurrent peaks increases with the decrease in atom-surface distance. The new feature is ascribed to the bifurcation of new closed orbits in the classical dynamics of the photoionized electron. Therefore, surface properties have a significant effect on the spectrum of nearby atoms or ions.%@@ The Ryderberg electronic wave packet dynamics of hydrogen atom near helium surface in an electric field is investigated using the semiclassical method.The autocorrelation function is calculated when the photoionized electron is excited by a short laser pulse for different atom-surface separations.The results show that new recurrences appear because of the helium surface, and the number of recurrent peaks increases with the decrease in atom-surface distance.The new feature is ascribed to the bifurcation of new closed orbits in the classical dynamics of the photoionized electron.Therefore, surface properties have a significant effect on the spectrum of nearby atoms or ions.

  3. Attenuation of vacuum ultraviolet light in liquid argon

    CERN Document Server

    Neumeier, A; Oberauer, L; Potzel, W; Schönert, S; Dandl, T; Heindl, T; Ulrich, A; Wieser, J

    2015-01-01

    The transmission of liquid argon has been measured, wavelength resolved, for a wavelength interval from 118 to 250 nm. The wavelength dependent attenuation length is presented for pure argon. It is shown that no universal wavelength independent attenuation length can be assigned to liquid argon for its own fluorescence light due to the interplay between the wavelength dependent emission and absorption. A decreasing transmission is observed below 130 nm in both chemically cleaned and distilled liquid argon and assigned to absorption by the analogue of the first argon excimer continuum. For not perfectly cleaned argon a strong influence of impurities on the transmission is observed. Two strong absorption bands at 126.5 and 141.0 nm with approximately 2 and 4 nm width, respectively, are assigned to traces of xenon in argon. A broad absorption region below 180 nm is found for unpurified argon and tentatively attributed to the presence of water in the argon sample.

  4. Anomalous argon excitation in pulse supersonic flows of Ar + CH sub 4 , Ar + SiH sub 4 and Ar + CH sub 4 + SiH sub 4 mixtures, activated with an electron beam

    CERN Document Server

    Madirbaev, V Z; Korobejshchikov, N G; Sharafutdinov, R G

    2001-01-01

    The processes of energy exchange in the supersonic flows of the argon mixtures with methane and silane, activated by the electron beam, are studied. It is shown, that at the initial stage of condensation in the flux there takes place selective excitation of the argon atoms energy levels. The boundary parameters, whereby the effect of the anomalous radiation excitation is observed, are determined

  5. Converging of Argon Cluster Ion Beams with a Glass Capillary

    Science.gov (United States)

    Shoji, Kazuhiro; Iuchi, Kensuke; Izumi, Motoki; Moritani, Kousuke; Inui, Norio; Mochiji, Kozo

    We have investigated the converging behavior of argon gas cluster ion beam passed through a glass capillary. The gas cluster ions are attractive as a projectile for SIMS from the view point of minimization of the damages. The cluster ion beam of 5 keV consisting of 500˜3000 argon atoms was injected in the capillary. The inner diameters of the capillary at the inlet and outlet were 0.8 mm and 9.6˜140 μm, respectively. Ion current from the outlet of the all the capillaries were detected. We obtained the converging factor of 2˜7, which depended on the incident ion current. The kinetic energy of the incident ions was found to be reduced by 20˜30% by passing through the capillary. Contrary, the velocity of the ions was not changed. These facts suggest that the cluster becomes 20˜30% smaller in mass by passing through the capillary. As far as we know, this is the first report on the study of the converging of cluster ions by using a glass capillary.

  6. Helium-Implantation-Induced Damage in NHS Steel Investigated by Slow-Positron Annihilation Spectroscopy

    Science.gov (United States)

    Li, Yuan-Fei; Shen, Tie-Long; Gao, Xing; Gao, Ning; Yao, Cun-Feng; Sun, Jian-Rong; Wei, Kong-Fang; Li, Bing-Sheng; Zhang, Peng; Cao, Xing-Zhong; Zhu, Ya-Bin; Pang, Li-Long; Cui, Ming-Huan; Chang, Hai-Long; Wang, Ji; Zhu, Hui-Ping; Wang, Dong; Song, Peng; Sheng, Yan-Bin; Zhang, Hong-Peng; Hu, Bi-Tao; Wang, Zhi-Guang

    2014-03-01

    Evolutions of defects and helium contained defects produced by atomic displacement and helium deposition with helium implantation at different temperatures in novel high silicon (NHS) steel are investigated by a slow positron beam. Differences of the defect information among samples implanted by helium to a fluence of 1 × 1017 ions/cm2 at room temperature, 300°C, 450°C and 750°C are discussed. It is found that the mobility of vacancies and vacancy clusters, a recombination of vacancy-type defects and the formation of the He-V complex lead to the occurrence of these differences. At high temperature irradiations, a change of the diffusion mechanism of He atoms/He bubbles might be one of the reasons for the change of the S-parameter.

  7. Limitations of superfluid helium droplets as host system revealed by electronic spectroscopy of embedded molecules

    Energy Technology Data Exchange (ETDEWEB)

    Premke, Tobias

    2016-02-19

    Superfluid helium nanodroplets serve a unique cryogenic host system ideal to prepare cold molecules and clusters. Structures as well as dynamic processes can be examined by means of high resolution spectroscopy. Dopant spectra are accompanied by helium-induced spectroscopic features which reveal information on the dopant to helium interaction. For this reason the experimental research focuses on the investigation of such helium-induced effects in order to provide new information on the microsolvation inside the droplets. Since the quantitative understanding of helium-induced spectral features is essential to interpret molecular spectra recorded in helium droplets, this study contributes further experimental details on microsolvation in superfluid helium droplets. For this purpose two contrary systems were examined by means of high resolution electronic spectroscopy. The first one, phthalocyanine (Pc), is a planar organic molecule offering a huge and planar surface to the helium atoms and thus, the non-superfluid helium solvation layer can form different structures. The second system is iodine and in contrast to Pc it is of simple molecular shape. That means that in this case different complex structures of the non-superfluid helium solvation layer and the dopant can be expected to be avoided. Thus, both molecules should show clear differences in their microsolvation behavior. In this work a detailed examination of different spectroscopic properties of phthalocyanine is given by means of fluorescence excitation and dispersed emission spectroscopy. It raises legitimate doubts about the assignment of experimentally observed signals to features predicted by the model of the microsolvation. Even though there are no experimental observations which disprove the empirical model for the solvation in helium droplets, an unambiguous assignment of the helium-induced spectroscopic structures is often not possible. In the second part of this work, the investigation of the

  8. EPR-Spin Trapping and Flow Cytometric Studies of Free Radicals Generated Using Cold Atmospheric Argon Plasma and X-Ray Irradiation in Aqueous Solutions and Intracellular Milieu.

    Directory of Open Access Journals (Sweden)

    Hidefumi Uchiyama

    Full Text Available Electron paramagnetic resonance (EPR-spin trapping and flow cytometry were used to identify free radicals generated using argon-cold atmospheric plasma (Ar-CAP in aqueous solutions and intracellularly in comparison with those generated by X-irradiation. Ar-CAP was generated using a high-voltage power supply unit with low-frequency excitation. The characteristics of Ar-CAP were estimated by vacuum UV absorption and emission spectra measurements. Hydroxyl (·OH radicals and hydrogen (H atoms in aqueous solutions were identified with the spin traps 5,5-dimethyl-1-pyrroline N-oxide (DMPO, 3,3,5,5-tetramethyl-1-pyrroline-N-oxide (M4PO, and phenyl N-t-butylnitrone (PBN. The occurrence of Ar-CAP-induced pyrolysis was evaluated using the spin trap 3,5-dibromo-4-nitrosobenzene sulfonate (DBNBS in aqueous solutions of DNA constituents, sodium acetate, and L-alanine. Human lymphoma U937 cells were used to study intracellular oxidative stress using five fluorescent probes with different affinities to a number of reactive species. The analysis and quantification of EPR spectra revealed the formation of enormous amounts of ·OH radicals using Ar-CAP compared with that by X-irradiation. Very small amounts of H atoms were detected whereas nitric oxide was not found. The formation of ·OH radicals depended on the type of rare gas used and the yield correlated inversely with ionization energy in the order of krypton > argon = neon > helium. No pyrolysis radicals were detected in aqueous solutions exposed to Ar-CAP. Intracellularly, ·OH, H2O2, which is the recombination product of ·OH, and OCl- were the most likely formed reactive oxygen species after exposure to Ar-CAP. Intracellularly, there was no practical evidence for the formation of NO whereas very small amounts of superoxides were formed. Despite the superiority of Ar-CAP in forming ·OH radicals, the exposure to X-rays proved more lethal. The mechanism of free radical formation in aqueous solutions and

  9. EPR-Spin Trapping and Flow Cytometric Studies of Free Radicals Generated Using Cold Atmospheric Argon Plasma and X-Ray Irradiation in Aqueous Solutions and Intracellular Milieu.

    Science.gov (United States)

    Uchiyama, Hidefumi; Zhao, Qing-Li; Hassan, Mariame Ali; Andocs, Gabor; Nojima, Nobuyuki; Takeda, Keigo; Ishikawa, Kenji; Hori, Masaru; Kondo, Takashi

    2015-01-01

    Electron paramagnetic resonance (EPR)-spin trapping and flow cytometry were used to identify free radicals generated using argon-cold atmospheric plasma (Ar-CAP) in aqueous solutions and intracellularly in comparison with those generated by X-irradiation. Ar-CAP was generated using a high-voltage power supply unit with low-frequency excitation. The characteristics of Ar-CAP were estimated by vacuum UV absorption and emission spectra measurements. Hydroxyl (·OH) radicals and hydrogen (H) atoms in aqueous solutions were identified with the spin traps 5,5-dimethyl-1-pyrroline N-oxide (DMPO), 3,3,5,5-tetramethyl-1-pyrroline-N-oxide (M4PO), and phenyl N-t-butylnitrone (PBN). The occurrence of Ar-CAP-induced pyrolysis was evaluated using the spin trap 3,5-dibromo-4-nitrosobenzene sulfonate (DBNBS) in aqueous solutions of DNA constituents, sodium acetate, and L-alanine. Human lymphoma U937 cells were used to study intracellular oxidative stress using five fluorescent probes with different affinities to a number of reactive species. The analysis and quantification of EPR spectra revealed the formation of enormous amounts of ·OH radicals using Ar-CAP compared with that by X-irradiation. Very small amounts of H atoms were detected whereas nitric oxide was not found. The formation of ·OH radicals depended on the type of rare gas used and the yield correlated inversely with ionization energy in the order of krypton > argon = neon > helium. No pyrolysis radicals were detected in aqueous solutions exposed to Ar-CAP. Intracellularly, ·OH, H2O2, which is the recombination product of ·OH, and OCl- were the most likely formed reactive oxygen species after exposure to Ar-CAP. Intracellularly, there was no practical evidence for the formation of NO whereas very small amounts of superoxides were formed. Despite the superiority of Ar-CAP in forming ·OH radicals, the exposure to X-rays proved more lethal. The mechanism of free radical formation in aqueous solutions and an

  10. Facile time-of-flight methods for characterizing pulsed superfluid helium droplet beams

    Energy Technology Data Exchange (ETDEWEB)

    He, Yunteng; Zhang, Jie; Li, Yang; Freund, William M.; Kong, Wei, E-mail: wei.kong@oregonstate.edu [Department of Chemistry, Oregon State University, Corvallis, Oregon 97331 (United States)

    2015-08-15

    We present two facile time-of-flight (TOF) methods of detecting superfluid helium droplets and droplets with neutral dopants. Without an electron gun and with only a heated filament and pulsed electrodes, the electron impact ionization TOF mass spectrometer can resolve ionized helium clusters such as He{sub 2}{sup +} and He{sub 4}{sup +}, which are signatures of superfluid helium droplets. Without ionizing any helium atoms, multiphoton non-resonant laser ionization of CCl{sub 4} doped in superfluid helium droplets at 266 nm generates complex cluster ions of dopant fragments with helium atoms, including (He){sub n}C{sup +}, (He){sub n}Cl{sup +}, and (He){sub n}CCl{sup +}. Using both methods, we have characterized our cryogenic pulsed valve—the Even-Lavie valve. We have observed a primary pulse with larger helium droplets traveling at a slower speed and a rebound pulse with smaller droplets at a faster speed. In addition, the pickup efficiency of dopant is higher for the primary pulse when the nozzle temperature is higher than 13 K, and the total time duration of the doped droplet pulse is only on the order of 20 μs. These results stress the importance of fast and easy characterization of the droplet beam for sensitive measurements such as electron diffraction of doped droplets.

  11. Facile time-of-flight methods for characterizing pulsed superfluid helium droplet beams.

    Science.gov (United States)

    He, Yunteng; Zhang, Jie; Li, Yang; Freund, William M; Kong, Wei

    2015-08-01

    We present two facile time-of-flight (TOF) methods of detecting superfluid helium droplets and droplets with neutral dopants. Without an electron gun and with only a heated filament and pulsed electrodes, the electron impact ionization TOF mass spectrometer can resolve ionized helium clusters such as He2(+) and He4(+), which are signatures of superfluid helium droplets. Without ionizing any helium atoms, multiphoton non-resonant laser ionization of CCl4 doped in superfluid helium droplets at 266 nm generates complex cluster ions of dopant fragments with helium atoms, including (He)(n)C(+), (He)(n)Cl(+), and (He)(n)CCl(+). Using both methods, we have characterized our cryogenic pulsed valve—the Even-Lavie valve. We have observed a primary pulse with larger helium droplets traveling at a slower speed and a rebound pulse with smaller droplets at a faster speed. In addition, the pickup efficiency of dopant is higher for the primary pulse when the nozzle temperature is higher than 13 K, and the total time duration of the doped droplet pulse is only on the order of 20 μs. These results stress the importance of fast and easy characterization of the droplet beam for sensitive measurements such as electron diffraction of doped droplets.

  12. Global model including multistep ionizations in helium plasmas

    Science.gov (United States)

    Oh, Seung-Ju; Lee, Hyo-Chang; Chung, Chin-Wook

    2016-12-01

    Particle and power balance equations including stepwise ionizations are derived and solved in helium plasmas. In the balance equations, two metastable states (21S1 in singlet and 23S1 triplet) are considered and the followings are obtained. The plasma density linearly increases and the electron temperature is relatively in a constant value against the absorbed power. It is also found that the contribution to multi-step ionization with respect to the single-step ionization is in the range of 8%-23%, as the gas pressure increases from 10 mTorr to 100 mTorr. Compared to the results in the argon plasma, there is little variation in the collisional energy loss per electron-ion pair created (ɛc) with absorbed power and gas pressure due to the small collision cross section and higher inelastic collision threshold energy.

  13. Molecular superfluidity in helium clusters studied using impulsive alignment

    Energy Technology Data Exchange (ETDEWEB)

    Galinis, Gediminas; Mendoza Luna, Luis Guillermo; Watkins, Mark; Von Haeften, Klaus [Department of Physics and Astronomy, University of Leicester (United Kingdom); Kazak, Lev; Goede, Sebastian; Skruszewicz, Slawomir; Irsig, Robert; Tiggesbaeumker, Josef; Meiwes-Broer, Karl-Heinz [Institut fuer Physik, Universitaet Rostock (Germany); Minns, Russell [Department of Chemistry, University of Southampton (United Kingdom); Ellis, Andrew [Department of Chemistry, University of Leicester (United Kingdom); Turcu, Edmon; Cacho, Cephise; Springate, Emma [CLF, STFC, Rutherford Appleton Laboratories (United Kingdom)

    2013-07-01

    Superfluidity is an intriguing phenomenon commonly associated with frictionless flow. Although this macroscopic effect is well understood, our understanding of how superfluidity evolves on the nanoscale is less extensive.We apply new approach to study superfluidity as a function of the number of helium atoms involved. A femtosecond pump-probe laser setup is used to excite a rotational wavepacket and to follow its propagation in time. The periodically recurring molecular alignment is probed by analyzing the emission characteristics in delayed Coulomb explosion with a velocity map imaging (VMI) spectrometer. First results show CO attached to five helium atoms and rotational features of HCCH-He corresponding to a linear configuration. To maximize the molecular beam intensity and to cope with the associated high gas load we developed a unique, differentially pumped VMI spectrometer.

  14. Diffusion Coefficient of Helium in Mo-Assessed by the Internal Friction Technique

    Institute of Scientific and Technical Information of China (English)

    WANG Weiguo; YANG Junfeng; WANG Xianping; XIE Chunyi; LI Renhong; CHEN Junling; FANG Qianfeng

    2009-01-01

    Diffusion behavior of helium in molybdenum was investigated by means of the in-ternal friction method. An apparent relaxation internal friction peak associated with helium long-range diffusion was observed around 475 K at a resonant frequency of 56 Hz. In terms of the Gorsky relaxation model and the shift of the peak position with the measurement frequency, the activation energy and pre-exponential factor of the diffusion coefficient of the helium atoms in molybdenum were deduced as 0.63 eV and 6.5 cm2/s, respectively.

  15. Development of a supercritical helium turbine; Chorinkaiatsu heriumu-tabin bochoki no kaihatsu

    Energy Technology Data Exchange (ETDEWEB)

    Kato, T.; Kawano, K.; Shinba, T.; Hiyama, T.; Tsuji, H. [Japan Atomic Energy Research Inst., Tokyo (Japan); Saji, N.; Asakura, H.; Yoshinaga, S. [Ishikawajima-Harima Heavy Industries Co., Ltd., Tokyo (Japan)

    1999-11-10

    The thermal efficiency of helium refrigerator is improved, and the adoption of supercritical pressure helium turbine expander which moves at entrance pressure 1.6MPa and 8-6K inlet temperature in which the JT's style is made to expand as the means in which refrigerating machine main body is miniaturized directly is mentioned. In the meantime, ability adjustment mechanism of the refrigerating machine is required, since the thermal load, which arises in superconducting coil for ITER, fluctuates. Then, Japan Atomic Energy Res. Inst., Ishikawajima-Harima Heavy Industries developed the supercritical pressure helium turbine expander with the capacity variable mechanism in the cooperation. (NEDO)

  16. Effect of argon during diamond deposition

    Energy Technology Data Exchange (ETDEWEB)

    Barbosa, D.C.; Mengui, U.A.; Contin, A.; Trava-Airoldi, V.J.; Baldan, M.R.; Corat, E.J. [Instituto Nacional de Pesquisas Espaciais (INPE), Sao Jose dos Campos, SP (Brazil). Laboratorio Associado de Sensores e Materiais

    2014-07-01

    The effect of argon content upon the growth rate and the properties of diamond thin films grown with different grains sizes is explored. An argon-free and argon-rich gas mixture of methane and hydrogen is used in a hot filament chemical vapor deposition reactor. Characterization of the films is accomplished by scanning electron microscopy, Raman spectroscopy and high-resolution x-ray diffraction. An extensive comparison of the growth rate values obtained in this study with those found in the literature suggests that there are distinct common trends for microcrystalline and nanocrystalline diamond growth, despite a large variation in the gas mixture composition. Included is a discussion of the possible reasons for these observations. (author)

  17. Summary of results from the TEXTOR helium self-pumping experiment

    Energy Technology Data Exchange (ETDEWEB)

    Brooks, J.N.; Krauss, A. [Argonne National Lab., IL (United States); Nygren, R.E.; Doyle, B.L. [Sandia National Labs., Albuquerque, NM (United States); Dippel, K.H.; Finken, K.H. [Association Euratom-Kernforschungsanlage Juelich (Germany). Inst. fuer Plasmaphysik

    1992-03-01

    Helium removal experiments were conducted in TEXTOR with a small helium self-pumping module located in a modified ALT-I limiter head. The module contained two heated nickel alloy trapping plates, a nickel deposition filament array, a Langmuir probe, flux probe, and thermocouples. The experiment examined plasma helium removal via trapping of helium ions in the deposited nickel surfaces. Such helium removal was successfully observed, with about 10% of the helium He/D plasma being removed in a {approximately}1 s period. The module was found to be compatible with overall tokamak operation with essentially no sputtered nickel entering the core plasma. The temperature rise on the ion-exposed inner trapping plate, during a plasma shot, is consistent with a nickel a local sheath potential of {approximately}3 kT{sub e}. Post-tokamak test examination of the trapping plates shows helium atom concentrations in the deposited nickel consistent with the observed helium removal, and shows very small D concentrations.

  18. Electron Neutrino Classification in Liquid Argon Time Projection Chamber Detector

    CERN Document Server

    Płoński, Piotr; Sulej, Robert; Zaremba, Krzysztof

    2015-01-01

    Neutrinos are one of the least known elementary particles. The detection of neutrinos is an extremely difficult task since they are affected only by weak sub-atomic force or gravity. Therefore large detectors are constructed to reveal neutrino's properties. Among them the Liquid Argon Time Projection Chamber (LAr-TPC) detectors provide excellent imaging and particle identification ability for studying neutrinos. The computerized methods for automatic reconstruction and identification of particles are needed to fully exploit the potential of the LAr-TPC technique. Herein, the novel method for electron neutrino classification is presented. The method constructs a feature descriptor from images of observed event. It characterizes the signal distribution propagated from vertex of interest, where the particle interacts with the detector medium. The classifier is learned with a constructed feature descriptor to decide whether the images represent the electron neutrino or cascade produced by photons. The proposed ap...

  19. Kinetic modeling of the Townsend breakdown in argon

    Energy Technology Data Exchange (ETDEWEB)

    Macheret, S. O.; Shneider, M. N. [Department of Mechanical and Aerospace Engineering, Princeton University, D-414 Engineering Quadrangle, Princeton, New Jersey 08544 (United States)

    2013-10-15

    Kinetic modeling of the Townsend breakdown in argon was performed in the “forward-back” approximation. The kinetic model was found to adequately describe the left branch of the Paschen curve, and the important role of ionization by fast ions and atoms near the cathode, as well as the increase in secondary emission coefficient in strong electric fields described in the literature, was confirmed. The modeling also showed that the electron energy distribution function develops a beam of high-energy electrons and that the runaway effect, i.e., the monotonic increase of the mean electron energy with the distance from the cathode, occurs at the left branch of the Paschen curve.

  20. Argon plasma immersion ion implantation of polystyrene films

    Energy Technology Data Exchange (ETDEWEB)

    Kondyurin, A. [Applied and Plasma Physics, School of Physics (A28), University of Sydney, New South Wales 2006 (Australia)], E-mail: kond@mailcity.com; Gan, B.K.; Bilek, M.M.M.; McKenzie, D.R.; Mizuno, K. [Applied and Plasma Physics, School of Physics (A28), University of Sydney, New South Wales 2006 (Australia); Wuhrer, R. [Microstructural Analysis Unit, University of Technology Sydney, P.O. Box 123, Broadway, NSW 2007 (Australia)

    2008-04-15

    Plasma immersion ion implantation (PIII), using bias voltages of 5, 10, 15 and 20 kV in an argon plasma and fluences in the range of 2 x 10{sup 14}-2 x 10{sup 16} ions/cm{sup 2}, was applied to 100 nm polystyrene films coated on silicon wafer substrates. The etching kinetics and structural changes induced in the polystyrene films were investigated with ellipsometry, Raman and FTIR spectroscopies, optical and scanning electron microscopies, atomic force microscopy and contact angle measurements. Effects such as carbonisation, oxidation and cross-linking were observed and their dependence on the applied bias voltage is reported. Variations in the etching rate during the PIII process and its relationship to carbonisation of the modified surface layer are explored.

  1. Studies on argon collisions with smooth and rough tungsten surfaces.

    Science.gov (United States)

    Ozhgibesov, M S; Leu, T S; Cheng, C H; Utkin, A V

    2013-09-01

    The aim of this work is to investigate argon scattering behaviors on the smooth and rough tungsten surfaces. Current work deals with numerical simulation of nanoscale heat transfer process accompanying with rarefied gas-solid substrate interactions using molecular dynamics (MD) method. Taking into account that this method is very time consuming, MD simulation using CUDA capable Graphic Cards is implemented. The results found that imperfection of the surface significantly influences on gas atom's momentum change upon collision. However, the energy exchange rate remains unchanged regardless to the surface roughness. This finding is in contrast with the results in extant literatures. We believed the results found in this paper are important for both numerical and theoretical analyses of rarefied gas flow in micro- and nano-systems where the choice of boundary conditions significantly influences flow.

  2. Novel nuclear laser spectroscopy method using superfluid helium for measurement of spins and moments of exotic nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Furukawa, Takeshi, E-mail: takeshi@tmu.ac.jp [Department of Physics, Tokyo Metropolitan University, 1-1 Minami-Osawa, Hachioji, Tokyo 192-0397 (Japan); RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Wakui, Takashi [Cyclotron and Radioisotope Center, Tohoku University, 6-3 Aoba, Aramaki, Aoba, Sendai, Miyagi 980-8578 (Japan); Yang, Xiaofei [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); School of Physics, Peking University, Chengfu Road, Haidian District, Beijing 100871 (China); Fujita, Tomomi [Department of Physics, Osaka University, 1-1 Machikaneyama, Toyonaka, Osaka 560-0043 (Japan); Imamura, Kei; Yamaguchi, Yasuhiro [Department of Physics, Meiji University, 1-1-1 Higashi-Mita, Tama, Kawasaki, Kanagawa 214-8571 (Japan); Tetsuka, Hiroki; Tsutsui, Yoshiki [Department of Physics, Tokyo Gakugei University, 4-1-1 Nukuikitamachi, Koganei, Tokyo 184-8501,Japan (Japan); Mitsuya, Yosuke [Department of Physics, Meiji University, 1-1-1 Higashi-Mita, Tama, Kawasaki, Kanagawa 214-8571 (Japan); Ichikawa, Yuichi [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Department of Physics, Tokyo Institute of Technology, 2-12-1 Ookayama, Meguro, Tokyo 152-8551 (Japan); Ishibashi, Yoko [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Department of Physics, University of Tsukuba, 1-1-1 Tennodai, Tsukuba, Ibaraki 305-8577 (Japan); Yoshida, Naoki; Shirai, Hazuki [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Department of Physics, Tokyo Institute of Technology, 2-12-1 Ookayama, Meguro, Tokyo 152-8551 (Japan); Ebara, Yuta; Hayasaka, Miki [Department of Physics, Tokyo Gakugei University, 4-1-1 Nukuikitamachi, Koganei, Tokyo 184-8501,Japan (Japan); Arai, Shino; Muramoto, Sosuke [Department of Physics, Meiji University, 1-1-1 Higashi-Mita, Tama, Kawasaki, Kanagawa 214-8571 (Japan); and others

    2013-12-15

    Highlights: • Development of a novel nuclear laser spectroscopy method using superfluid helium. • Observation of the Zeeman resonance with the {sup 85}Rb beam introduced into helium. • Demonstration of deducing the nuclear spins from the observed resonance spectrum. -- Abstract: We have been developing a novel nuclear laser spectroscopy method “OROCHI” for determining spins and moments of exotic radioisotopes. In this method, we use superfluid helium as a stopping material of energetic radioisotope beams and then stopped radioisotope atoms are subjected to in situ laser spectroscopy in superfluid helium. To confirm the feasibility of this method for rare radioisotopes, we carried out a test experiment using a {sup 85}Rb beam. In this experiment, we have successfully measured the Zeeman resonance signals from the {sup 85}Rb atoms stopped in superfluid helium by laser-RF double resonance spectroscopy. This method is efficient for the measurement of spins and moments of more exotic nuclei.

  3. ICARUS and status of liquid argon technology

    CERN Document Server

    Menegolli, Alessandro

    2012-01-01

    ICARUS T600 is the largest liquid Argon Time Projection Chamber (LAr TPC) detector ever realized. It operates underground at the LNGS laboratory in Gran Sasso. It has been smoothly running since summer 2010, collecting data with the CNGS (Cern to Gran Sasso) beam and with cosmic particles. Liquid Argon TPCs are indeed 'electronic bubble chambers', providing a completely uniform imaging calorimetry with unprecedented accuracy on such massive volumes. ICARUS T600 is internationally considered as a milestone towards the realization of the next generation of massive detectors (tens of ktons) for neutrino and rare event physics. Results will be presented on the data collected so far with the detector.

  4. Neutrons on a surface of liquid helium

    Science.gov (United States)

    Grigoriev, P. D.; Zimmer, O.; Grigoriev, A. D.; Ziman, T.

    2016-08-01

    We investigate the possibility of ultracold neutron (UCN) storage in quantum states defined by the combined potentials of the Earth's gravity and the neutron optical repulsion by a horizontal surface of liquid helium. We analyze the stability of the lowest quantum state, which is most susceptible to perturbations due to surface excitations, against scattering by helium atoms in the vapor and by excitations of the liquid, comprised of ripplons, phonons, and surfons. This is an unusual scattering problem since the kinetic energy of the neutron parallel to the surface may be much greater than the binding energies perpendicular. The total scattering time of these UCNs at 0.7 K is found to exceed 1 h, and rapidly increases with decreasing temperature. Such low scattering rates should enable high-precision measurements of the sequence of discrete energy levels, thus providing improved tests of short-range gravity. The system might also be useful for neutron β -decay experiments. We also sketch new experimental propositions for level population and trapping of ultracold neutrons above a flat horizontal mirror.

  5. Neutrons on a surface of liquid helium

    CERN Document Server

    Grigoriev, P D; Ziman, T; Grigoriev, A D

    2015-01-01

    We investigate the possibility of ultracold neutron (UCN) storage in quantum states defined by the combined potentials of the Earth's gravity and the neutron optical repulsion by a horizontal surface of liquid helium. We analyse the stability of the lowest quantum state, which is most susceptible to perturbations due to surface excitations, against scattering by helium atoms in the vapor and by excitations of the liquid, comprised of ripplons, phonons and surfons. This is an unusual scattering problem since the kinetic energy of the neutron parallel to the surface may be much greater than the binding energies perpendicular. The total scattering time constant of these UCNs at 0.7 K is found to exceed one hour, and rapidly increasing with decreasing temperature. Such low scattering rates should enable high-precision measurements of the scheme of discrete energy levels, thus providing improved access to short-range gravity. The system might also be useful for neutron beta-decay experiments. We also sketch new ex...

  6. Effective potentials for charge-helium and charge-singly-ionized helium interactions in a dense plasma

    Energy Technology Data Exchange (ETDEWEB)

    Ramazanov, T.S.; Amirov, S.M.; Moldabekov, Zh.A. [Institute for Experimental and Theoretical Physics, Al-Farabi Kazakh National University, Almaty (Kazakhstan)

    2016-06-15

    The effective electron (proton)-He and electron (proton)-He{sup +} screened pair interaction potentials arising as a result of partial screening of the helium nucleus field by bound electrons, taking into account both screening by free charged particles and quantum diffraction effect in dense plasmas were derived. The impact of quantum effects on screening was analyzed. It was shown that plasma polarization around the atom leads to the additional repulsion (attraction) between the electron (proton) and the helium atom. The method of constructing the full electron (proton)-He and electron (proton)-He{sup +} screened pair interaction potentials as the sum of the derived potentials with the polarization potential and exchange potential is discussed. (copyright 2016 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  7. Hf impurity and defect interactions in helium-implanted NiHf

    Energy Technology Data Exchange (ETDEWEB)

    Govindaraj, R. E-mail: govind@igcar.ernet.in; Gopinathan, K.P.; Viswanathan, B

    2001-07-01

    TDPAC measurements on the reference and untreated sample indicate a loss in anisotropy which is attributed mainly to the association of probe atoms with defects produced by (n,{gamma}) reactions with isotopes of Ni and experiencing combined magnetic and quadrupole interactions of comparable strengths. Evolution of defect free and substitutional fraction of probe atoms experiencing Larmor frequency characteristic of Ni matrix has been studied as a function of isochronal annealing temperature in helium free {alpha}-irradiated and homogeneously helium-implanted samples. No defect associated Larmor precession frequency and/or quadrupole frequency could be deduced in these uncorrelated damage studies. Comparison of recovery stages in {alpha}-irradiated and helium-implanted samples indicates the binding of helium associated defects by Hf impurities. Segregation of Hf atoms is observed in the helium free {alpha}-irradiated sample for annealing treatment at 973 K, while no such effect is observed in the helium-implanted sample for isochronal annealing treatments up to 1273 K.

  8. ITER helium ash accumulation

    Energy Technology Data Exchange (ETDEWEB)

    Hogan, J.T.; Hillis, D.L.; Galambos, J.; Uckan, N.A. (Oak Ridge National Lab., TN (USA)); Dippel, K.H.; Finken, K.H. (Forschungszentrum Juelich GmbH (Germany, F.R.). Inst. fuer Plasmaphysik); Hulse, R.A.; Budny, R.V. (Princeton Univ., NJ (USA). Plasma Physics Lab.)

    1990-01-01

    Many studies have shown the importance of the ratio {upsilon}{sub He}/{upsilon}{sub E} in determining the level of He ash accumulation in future reactor systems. Results of the first tokamak He removal experiments have been analysed, and a first estimate of the ratio {upsilon}{sub He}/{upsilon}{sub E} to be expected for future reactor systems has been made. The experiments were carried out for neutral beam heated plasmas in the TEXTOR tokamak, at KFA/Julich. Helium was injected both as a short puff and continuously, and subsequently extracted with the Advanced Limiter Test-II pump limiter. The rate at which the He density decays has been determined with absolutely calibrated charge exchange spectroscopy, and compared with theoretical models, using the Multiple Impurity Species Transport (MIST) code. An analysis of energy confinement has been made with PPPL TRANSP code, to distinguish beam from thermal confinement, especially for low density cases. The ALT-II pump limiter system is found to exhaust the He with maximum exhaust efficiency (8 pumps) of {approximately}8%. We find 1<{upsilon}{sub He}/{upsilon}{sub E}<3.3 for the database of cases analysed to date. Analysis with the ITER TETRA systems code shows that these values would be adequate to achieve the required He concentration with the present ITER divertor He extraction system.

  9. A G/NARRLI Effort. Measuring the Ionization Yield of Low-Energy Nuclear Recoils in Liquid Argon

    Energy Technology Data Exchange (ETDEWEB)

    Joshi, Tenzing Henry Yatish [Univ. of California, Berkeley, CA (United States)

    2014-01-01

    Liquid argon has long been used for particle detection due to its attractive drift properties, ample abundance, and reasonable density. The response of liquid argon to lowenergy O(102 -1044 eV) interactions is, however, largely unexplored. Weakly interacting massive particles such as neutrinos and hypothetical dark-matter particles (WIMPs) are predicted to coherently scatter on atomic nuclei, leaving only an isolated low-energy nuclear recoil as evidence. The response of liquid argon to low-energy nuclear recoils must be studied to determine the sensitivity of liquid argon based detectors to these unobserved interactions. Detectors sensitive to coherent neutrino-nucleus scattering may be used to monitor nuclear reactors from a distance, to detect neutrinos from supernova, and to test the predicted behavior of neutrinos. Additionally, direct detection of hypothetical weakly interacting dark matter would be a large step toward understanding the substance that accounts for nearly 27% of the universe. In this dissertation I discuss a small dual-phase (liquid-gas) argon proportional scintillation counter built to study the low-energy regime and several novel calibration and characterization techniques developed to study the response of liquid argon to low-energy O(102 -104 eV) interactions.

  10. Solar wind helium, neon and argon released by oxidation of metal grains from the Weston chondrite

    Science.gov (United States)

    Becker, R. H.; Rajan, R. S.; Rambaldi, E. R.

    1986-01-01

    A set of experiments were carried out to test the feasibility of determining unfractionated elemental and isotopic ratios for the noble gases in the presumably ancient solar wind present in the gas rich meteorites. The problems of diffusive loss was avoided by analyzing metal rather than the usual silicates. In order to avoid chemical, and even harsh physical, treatment of the sample, which might have affected the surfaces of metal grains, a means of analyzing the metal in the presence of residual silicate not removed by gentle crushing and magnetic separation was devised. Preliminary results given were obtained by taking advantage of the differing properties of metal and silicates with regard to diffusion. The results suggests that, with some modifications in the choice of pyrolysis and combustion temperatures and in the amount of O2 used, it should be possible, by oxidizing the surfaces of metal grains from gas rich meteorites, to obtain data on solar wind that has not been fractionated by diffusive loss.

  11. Helium 2 3S - 2 1S metrology at 1557 nm

    CERN Document Server

    Van Leeuwen, K A H

    2006-01-01

    An experiment is proposed to excite the 'forbidden' 1s2s 3S1 - 1s2s 1S0 magnetic dipole (M1) transition at 1557 nm in a collimated and slow atomic beam of metastable helium atoms. It is demonstrated that an excitation rate of 5000 /s can be realised with the beam of a 2W narrowband telecom fiber laser intersecting the atomic beam perpendicularly. A Doppler-limited sub-MHz spectroscopic linewidth is anticipated. Doppler-free excitation of 2% of trapped and cooled atoms may be realised in a one-dimensional optical lattice geometry, using the 2W laser both for trapping and spectroscopy. The very small (8 Hz) natural linewidth of this transition presents an opportunity for accurate tests of atomic structure calculations of the helium atom. A measurement of the 3He - 4He isotope shift allows for accurate determination of the difference in nuclear charge radius of both isotopes.

  12. Diffusion of helium in the perfect and non perfect uranium dioxide crystals and their local structures

    Energy Technology Data Exchange (ETDEWEB)

    Dabrowski, Ludwik, E-mail: luddab@hotmail.com; Szuta, Marcin

    2014-12-05

    Highlights: • The nano local structure of UO{sub 2} containing oxygen and uranium vacancies was identified. • We have determined for the first time in the UO{sub 2} the dynamical energy barriers to He migration. • It was found that the migration of helium is along the polylines. • The helium diffusion is accompanied of the emission–absorption of phonons. - Abstract: Local nano structures and their changes relevant with the diffusion of helium was determined by applying the density functional theory (DFT). With its help we calculated deformation of the crystal lattice while wandering helium atoms between octahedral sites. The optimal mutual coordinates of the atoms were determined by minimizing the Hellman–Feyman forces, allowing at the same time precisely specify dynamic height and the shape of the potential barrier. For a crystal containing single oxygen or uranium vacancies, has been described both the deformation associated with the presence of vacancy, as well as additional deformation related to the migration of the helium atom in the lattice. It was found that in the case of vacancies, the migration of helium atoms between the octahedral sites is not along a straight line but along a polyline. In addition, the presence of uranium vacancy causes that helium atoms in the octahedral sites, situated in the I and II coordination shell of uranium vacancy, have different energies. Migration between such positions must be carried out with the participation of the emission–absorption of phonons. Applying two site – model we evaluated the time for an over-barrier jump and diffusion of interstitial He. The obtained values for diffusion coefficient are compared with the experimentally obtained values and with the theoretical values of other authors.

  13. An Update of the Primordial Helium Abundance

    Science.gov (United States)

    Peimbert, Antonio; Peimbert, Manuel; Luridiana, Valentina

    2015-08-01

    Three of the best determinations of the primordial helium abundance (Yp) are those obtained from low metallicity HII regions by Aver, Olive, Porter, & Skillman (2013); Izotov, Thuan, & Guseva (2014); and Peimbert, Peimbert, & Luridiana (2007). In this poster we update the Yp determination by Peimbert et al. taking into account, among other aspects, recent advances in the determination of the He atomic physical parameters, the temperature structure, the collisional effects of high temperatures on the Balmer lines, as well as the effect of H and He bound-bound absorption.We compare our results with those of Aver et al. and Izotov et al. and point out possible explanations for the differences among the three determinations. We also compare our results with those obtained with the Plank satellite considering recent measurements of the neutron mean life; this comparison has implications on the determination of the number of light neutrino families.

  14. The primordial helium abundance from updated emissivities

    CERN Document Server

    Aver, Erik; Porter, R L; Skillman, Evan D

    2013-01-01

    Observations of metal-poor extragalactic H II regions allow the determination of the primordial helium abundance, Y_p. The He I emissivities are the foundation of the model of the H II region's emission. Porter, Ferland, Storey, & Detisch (2012) have recently published updated He I emissivities based on improved photoionization cross-sections. We incorporate these new atomic data and update our recent Markov Chain Monte Carlo analysis of the dataset published by Izotov, Thuan, & Stasinska (2007). As before, cuts are made to promote quality and reliability, and only solutions which fit the data within 95% confidence level are used to determine the primordial He abundance. The previously qualifying dataset is almost entirely retained and with strong concordance between the physical parameters. Overall, an upward bias from the new emissivities leads to a decrease in Y_p. In addition, we find a general trend to larger uncertainties in individual objects (due to changes in the emissivities) and an increase...

  15. Radiative corrections to the polarizability of helium.

    Science.gov (United States)

    Łach, Grzegorz; Jeziorski, Bogumił; Szalewicz, Krzysztof

    2004-06-11

    The complete alpha(3) QED correction to the helium atom polarizability is computed assuming an infinite nuclear mass and found to be equal to 0.000030666(3) a.u., with the contribution from the electric-field dependence of the Bethe logarithm amounting to 0.000000193(2) a.u. After including the alpha(2) and alpha(3) corrections for the nuclear recoil and the leading part of the alpha(4) QED correction, we find that the molar polarizability of 4He is 0.51725419(9)(4) cm(3)/mol. The first of the two error bounds is dominated by the uncertainty of alpha(4) and higher-order QED corrections and the second reflects the uncertainty of the Avogadro constant.

  16. Photoionization of helium dimers; Photoionisation von Heliumdimeren

    Energy Technology Data Exchange (ETDEWEB)

    Havermeier, Tilo

    2010-06-09

    The helium dimer is one of the most weakly bound systems in the universe. This makes it an interesting quantum mechanical object for investigation. These Van der Waals Clusters can be produced in an expansion of a cryogenic gas jet through a small nozzle into vacuum. In the present experiment we examine the interaction of He dimers with synchrotron radiation at an energy range from 64 to 78 eV. We observed different pathways leading to single ionization of both He atoms of the dimer compound. This two close standing ions begin now to dissociate in cause of their coulomb potential. All charged fragments were detected in coincidence with a COLTRIMS system. Especially Interatomic Coulombic Decay (ICD) and the two step process (TS1) were clearly identified. Furthermore a distribution of the internuclear distance was obtained from the measured Kinetic Energy Release (KER). (orig.)

  17. Modification on graphite due to helium ion irradiation

    Energy Technology Data Exchange (ETDEWEB)

    Dutta, N.J.; Mohanty, S.R., E-mail: smrutirm@yahoo.com; Buzarbaruah, N.

    2016-07-29

    This paper studies the influence of helium ion irradiation on morphological and structural properties of graphite samples. The helium ions emanated from a plasma focus device have been used to irradiate graphite samples by varying the number of ion pulses. The effect of radiation induced changes in morphology and structure are examined by using optical microscopy, atomic force microscopy, transmission electron microscopy along with selected area electron diffraction and x-ray diffraction. A distinct change in the surface topography is marked in the case of the ion irradiated samples when viewed under the optical microscope. The micrographs of the ion irradiated samples confirm mostly rounded and sparely elongated type of structures arising due to intense melting and local ablation accompanied with ejection of graphite melts that depends upon the ion fluence. The atomic force microscopy images also reveal the formation of globules having sizes ∼50–200 nm which are the agglomeration of small individual clusters. Transmission electron micrographs of the ion irradiated samples furnish that the diameter of these individual small clusters are ∼10.4 nm. Moreover, selected area electron diffraction patterns corroborate that the ion irradiated sample retains its crystalline nature, even after exposure to larger helium ion pulses. It is noticed from the x-ray diffraction patterns that some new phases are developed in the case of ion irradiated sample. - Highlights: • Used an ingenious helium ion source to study irradiation induced transformation on graphite. • OM, AFM and TEM analyses confirm the formation mostly rounded structures. • SAED patterns confirm the retention of crystallinity of graphite even after exposure to larger helium ion fluences. • XRD patterns confirm the development of new peaks that indicate structural rearrangement.

  18. Growing ultracold sodium clusters by using helium nanodroplets

    Science.gov (United States)

    Vongehr, S.; Scheidemann, A. A.; Wittig, C.; Kresin, V. V.

    2002-02-01

    The aggressive doping of helium droplets (˜10 5 atoms) with sodium vapor results in the growth of sodium clusters having up to at least 13 atoms, as determined by a Penning ionization technique. Signatures of electronic shell effects are observed in Na k+ cluster ions, including an odd-even intensity oscillation and an enhanced Na 9+ peak, which is a magic number effect. The size distributions are consistent with cluster ion fragmentation rather than simply sequential pickup statistics. The dependence of ion yield on mean ionizing electron energy suggests that neutral alkali clusters are located preferentially on the droplet surfaces.

  19. Positive and negative pulsed corona in argon

    NARCIS (Netherlands)

    Veldhuizen, E.M. van; Rutgers, W.R.; Ebert, U.

    2002-01-01

    Photographs are obtained of corona discharges in argon at atmospheric pressure using a high resolution, intensified CCD camera. Positive and negative polarity is applied at the curved electrode in a point-plane gap and a plane-plane gap with a protruding point. Branching is observed in the positive

  20. Thermal decomposition of barium valerate in argon

    DEFF Research Database (Denmark)

    Torres, P.; Norby, Poul; Grivel, Jean-Claude

    2015-01-01

    The thermal decomposition of barium valerate (Ba(C4H9CO2)(2)/Ba-pentanoate) was studied in argon by means of thermogravimetry, differential thermal analysis, IR-spectroscopy, X-ray diffraction and hot-stage optical microscopy. Melting takes place in two different steps, at 200 degrees C and 280...

  1. Cryogenic separation of an oxygen-argon mixture in natural air samples for the determination of isotope and molecular ratios.

    Science.gov (United States)

    Keedakkadan, Habeeb Rahman; Abe, Osamu

    2015-04-30

    The separation and purification of oxygen-argon mixtures are critical in the high-precision analysis of Δ(17) O and δ(O2 /Ar) for geochemical applications. At present, chromatographic methods are used for the separation and purification of oxygen-argon mixtures or pure oxygen, but these methods require the use of high-purity helium as a carrier gas. Considerable interest has been expressed in the development of a helium-free cryogenic separation of oxygen-argon mixtures in natural air samples. The precise and simplified cryogenic separation of oxygen-argon mixtures from natural air samples presented here was made possible using a single 5A (30/60 mesh) molecular sieve column. The method involves the trapping of eluted gases using molecular sieves at liquid nitrogen temperature, which is associated with isotopic fractionation. We tested the proposed method for the determination of isotopic fractionations during the gas exchange between water and atmospheric air at equilibrium. The dependency of fractionation was studied at different water temperatures and for different methods of equilibration (bubbling and stirring). Isotopic and molecular fractionations during gas desorption from molecular sieves were studied for different amounts and types of molecular sieves. Repeated measurements of atmospheric air yielded a reproducibility (±SD) of 0.021 ‰, 0.044 ‰, 15 per meg and 1.9 ‰ for δ(17) O, δ(18) O, Δ(17) O and δ(O2 /Ar) values, respectively. We applied the method to determine equilibrium isotope fractionation during gas exchange between air and water. Consistent δ(18) O and Δ(17) O results were obtained with the latest two studies, whereas there was a significant difference in δ(18) O values between seawater and deionized water. We have revised a helium-free, cryogenic separation of oxygen-argon mixtures in natural air samples for isotopic and molecular ratio analysis. The use of a single 13X (1/8" pellet) molecular sieve yielded the smallest isotopic

  2. 46 CFR 151.50-36 - Argon or nitrogen.

    Science.gov (United States)

    2010-10-01

    ... 46 Shipping 5 2010-10-01 2010-10-01 false Argon or nitrogen. 151.50-36 Section 151.50-36 Shipping... BULK LIQUID HAZARDOUS MATERIAL CARGOES Special Requirements § 151.50-36 Argon or nitrogen. (a) A cargo tank that contains argon or nitrogen and that has a maximum allowable working pressure of 172 kPa...

  3. Super-Maxwellian helium evaporation from pure and salty water.

    Science.gov (United States)

    Hahn, Christine; Kann, Zachary R; Faust, Jennifer A; Skinner, J L; Nathanson, Gilbert M

    2016-01-28

    Helium atoms evaporate from pure water and salty solutions in super-Maxwellian speed distributions, as observed experimentally and modeled theoretically. The experiments are performed by monitoring the velocities of dissolved He atoms that evaporate from microjets of pure water at 252 K and 4-8.5 molal LiCl and LiBr at 232-252 K. The average He atom energies exceed the flux-weighted Maxwell-Boltzmann average of 2RT by 30% for pure water and 70% for 8.5m LiBr. Classical molecular dynamics simulations closely reproduce the observed speed distributions and provide microscopic insight into the forces that eject the He atoms from solution. Comparisons of the density profile and He kinetic energies across the water-vacuum interface indicate that the He atoms are accelerated by He-water collisions within the top 1-2 layers of the liquid. We also find that the average He atom kinetic energy scales with the free energy of solvation of this sparingly soluble gas. This free-energy difference reflects the steeply decreasing potential of mean force on the He atoms in the interfacial region, whose gradient is the repulsive force that tends to expel the atoms. The accompanying sharp decrease in water density suppresses the He-water collisions that would otherwise maintain a Maxwell-Boltzmann distribution, allowing the He atom to escape at high energies. Helium is especially affected by this reduction in collisions because its weak interactions make energy transfer inefficient.

  4. Super-Maxwellian helium evaporation from pure and salty water

    Energy Technology Data Exchange (ETDEWEB)

    Hahn, Christine; Kann, Zachary R.; Faust, Jennifer A.; Skinner, J. L., E-mail: skinner@chem.wisc.edu, E-mail: nathanson@chem.wisc.edu; Nathanson, Gilbert M., E-mail: skinner@chem.wisc.edu, E-mail: nathanson@chem.wisc.edu [Department of Chemistry, University of Wisconsin-Madison, 1101 University Avenue, Madison, Wisconsin 53706 (United States)

    2016-01-28

    Helium atoms evaporate from pure water and salty solutions in super-Maxwellian speed distributions, as observed experimentally and modeled theoretically. The experiments are performed by monitoring the velocities of dissolved He atoms that evaporate from microjets of pure water at 252 K and 4–8.5 molal LiCl and LiBr at 232–252 K. The average He atom energies exceed the flux-weighted Maxwell-Boltzmann average of 2RT by 30% for pure water and 70% for 8.5m LiBr. Classical molecular dynamics simulations closely reproduce the observed speed distributions and provide microscopic insight into the forces that eject the He atoms from solution. Comparisons of the density profile and He kinetic energies across the water-vacuum interface indicate that the He atoms are accelerated by He–water collisions within the top 1-2 layers of the liquid. We also find that the average He atom kinetic energy scales with the free energy of solvation of this sparingly soluble gas. This free-energy difference reflects the steeply decreasing potential of mean force on the He atoms in the interfacial region, whose gradient is the repulsive force that tends to expel the atoms. The accompanying sharp decrease in water density suppresses the He–water collisions that would otherwise maintain a Maxwell-Boltzmann distribution, allowing the He atom to escape at high energies. Helium is especially affected by this reduction in collisions because its weak interactions make energy transfer inefficient.

  5. Pulse Shape Discrimination in liquid argon and its implications for Dark Matter searches using depleted argon

    CERN Document Server

    Kryczynski, Pawel

    2012-01-01

    A brief outline of Dark Matter detection experiments using liquid argon technology is presented. The Pulse Shape background discrimination method (PSD) is described and the example of its use in 2.3 l R&D detector is given. Methods of calculating sensitivity of a Dark Matter detector are discussed and used to estimate the possible improvement of sensitivity after introduction of isotopically depleted liquid argon.

  6. Observations of Lunar Exospheric Helium with LAMP UV Spectrograph onboard the Lunar Reconnaissance Orbiter

    Science.gov (United States)

    Grava, Cesare; Hurley, Dana M.; Retherford, Kurt D.; Gladstone, G. Randall; Feldman, Paul D.; Pryor, Wayne R.; Greathouse, Thomas K.; Mandt, Kathleen E.

    2017-04-01

    Helium was one of the first elements discovered in the lunar exosphere, being detected by the mass spectrometer LACE (Lunar Atmosphere Composition Experiment) deployed at the lunar surface during the Apollo 17 mission. Most of it comes from neutralization of solar wind alpha particles impinging on the lunar surface, but there is increasing evidence that a non-negligible fraction of it diffuses from the interior of the Moon, as a result of radioactive decay of thorium and uranium. Therefore, pinpointing the amount of endogenic helium can constrain the abundance of these two elements in the crust, with implication for the formation of the Moon. The Lyman-Alpha Mapping Project (LAMP) far-UV spectrograph onboard the Lunar Reconnaissance Orbiter (LRO) carried out an atmospheric campaign to study the lunar exospheric helium. The spacecraft was pitched along the direction of motion to look through a longer illuminated column of gas, compared to the usual nadir-looking mode, and therefore enhancing the brightness of the emission line at 58.4 nm of helium atoms resonantly scattering solar photons. The lines of sight of the observations spanned a variety of local times, latitudes, longitudes, and altitudes, allowing us to reconstruct the temporal and spatial distribution of helium and its radial density profile with the help of an exospheric model. Moreover, correlating the helium density inferred by LAMP with the flux of solar wind alpha particles (the main source of lunar helium) measured from the twin ARTEMIS spacecraft, it is possible to constrain the amount of helium which comes from the interior of the Moon via outgassing. While most of the observations can be explained by the exospheric model, we have found discrepancies between the model and LAMP observations, with the former underestimating the latter, especially at northern selenographic latitudes, when LRO altitude is maximum. Such discrepancies suggest that the vertical distribution of helium differs from a

  7. The second Born approximation of electron-argon elastic scattering in a Bichromatic laser field

    CERN Document Server

    Zhou, Bin; Wen, Da-Yong

    2013-01-01

    We study the elastic scattering of atomic argon by electron in the presence of a bichromatic laser field in the second Born approximation. The target atom is approximated by a simple screening potential and the continuum states of the impinging and emitting electrons are described as Volkov states. We evaluate the S-matrix elements numerically. The dependence of differential cross section on the relative phase between the two laser components is presented. The results obtained in the first and second Born approximation are compared and analysed.

  8. Bed system performance in helium circulation mode

    Energy Technology Data Exchange (ETDEWEB)

    Kim, Yean Jin; Jung, Kwang Jin; Ahn, Do Hee; Chung, Hong Suk [UST, Daejeon (Korea, Republic of); Kang, Hee Suk [KAERI, Daejeon (Korea, Republic of); Yun, Sei Hun [NFRI, Deajeon (Korea, Republic of)

    2016-05-15

    As a part of the International Thermonuclear Experimental Reactor (ITER) Project, We have conducted an experiment for storing hydrogen to depleted uranium and zirconium cobalt. The helium blanket effect has been observed in experiments using metal hydrides. The collapse of the hydrogen isotopes are accompanied by the decay heat and helium-3. Helium-3 dramatically reduces the hydrogen isotope storage capacity by surrounding the metal. This phenomenon is called a helium blanket effect. In addition the authors are working on the recovery and removal techniques of helium-3. In this paper, we discuss the equipment used to test the helium blanket effect and the results of a helium circulation experiment. The helium-3 produced surrounds the storage material surface and thus disturbs the reaction of the storage material and the hydrogen isotope. Even if the amount of helium-3 is small, the storage capacity of the SDS bed significantly drops. This phenomenon is the helium blanket effect. To resolve this phenomenon, a circulating loop was introduced. Using a circulating system, helium can be separated from the storage material. We made a helium loop that includes a ZrCo bed. Then using a metal bellows pump, we tested the helium circulation.

  9. Apparatus to measure low level helium for neutron dosimetry

    Energy Technology Data Exchange (ETDEWEB)

    Ozaki, Shuji; Takao, Yoshiyuki; Muramasu, Masatomo; Hida, Tomoya; Sou, Hirofumi; Nakashima, Hideki [Kyushu Univ., Fukuoka (Japan); Kanda, Yukinori

    1998-03-01

    An apparatus to measure low level helium in a solid sample for neutron dosimetry in the practical use such as area monitoring in the long-term and reactor surveillance was reported. In our previous work, the helium atoms measurement system (HAMS) was developed. A sample was evaporated in the furnace and the released gas from the sample was analyzed with the mass spectrometer of the system to determine the amount of helium contained in it. The system has been improved to advance the lower helium measurement limit in a solid sample for its application to an area monitoring system. The mass of a solid is up to 100mg. Two important points should be considered to advance the lower limit. One was to produce a high quality vacuum in the system chamber for suppressing background gases during the sample measurement. The other important point was to detect very small output from the mass spectrometer. A pulse counting system was used to get high sensitivity in the mass 4 analyzing. (author)

  10. Rogue mantle helium and neon.

    Science.gov (United States)

    Albarède, Francis

    2008-02-15

    The canonical model of helium isotope geochemistry describes the lower mantle as undegassed, but this view conflicts with evidence of recycled material in the source of ocean island basalts. Because mantle helium is efficiently extracted by magmatic activity, it cannot remain in fertile mantle rocks for long periods of time. Here, I suggest that helium with high 3He/4He ratios, as well as neon rich in the solar component, diffused early in Earth's history from low-melting-point primordial material into residual refractory "reservoir" rocks, such as dunites. The difference in 3He/4He ratios of ocean-island and mid-ocean ridge basalts and the preservation of solar neon are ascribed to the reservoir rocks being stretched and tapped to different extents during melting.

  11. Planar Rayleigh scattering results in helium-air mixing experiments in a Mach-6 wind tunnel

    Science.gov (United States)

    Shirinzadeh, B.; Hillard, M. E.; Balla, R. J.; Waitz, I. A.; Anders, J. B.; Exton, R. J.

    1992-01-01

    Planar Rayleigh scattering measurements with an argon-fluoride excimer laser are performed to investigate helium mixing into air at supersonic speeds. The capability of the Rayleigh scattering technique for flow visualization of a turbulent environment is demonstrated in a large-scale, Mach-6 facility. The detection limit obtained with the present setup indicates that planar, quantitative measurements of density can be made over a large cross-sectional area (5 cm x 10 cm) of the flow field in the absence of clusters.

  12. Charge and Energy Dependences of Ionization and Transfer for Helium in Collisions with Fast Charged Projectiles

    Institute of Scientific and Technical Information of China (English)

    FU Hong-Bin; WANG Bao-Hong; DING Bao-Wei; LIU Zhao-Yuan

    2009-01-01

    The classical method within the independent electron model is employed to investigate (i) charge dependences of single and double ionization for helium by various charged ions Aq+ (q = 1 - 8) at impact energies of 0.64 and 1.44 MeV/u, respectively, (ii) energy dependences of transfer ionization for helium by 0.5-3 MeV/u A8,9+ ions impact. The Lenz-Jensen model of the atom is applied instead of the Bohr model of the atom, and the impact-parameter dependences are also introduced into the calculations. Satisfactory agreement is found between theoretical and experimental data.

  13. Breit-Pauli and direct perturbation theory calculations of relativistic helium polarizability.

    Science.gov (United States)

    Cencek, W; Szalewicz, K; Jeziorski, B

    2001-06-18

    Large Gaussian-type geminal wave function expansions and direct perturbation theory (DPT) of relativistic effects have been applied to calculate the relativistic contribution to the static dipole polarizability of the helium atom. It has been demonstrated that DPT is superior for this purpose to traditional Breit-Pauli calculations. The resulting value of the molar polarizability of 4He is 0.517254(1) cm3 x mol(-1), including a literature estimate of QED effects. As a by-product, a very accurate value of the nonrelativistic helium second hyperpolarizability, gamma = 43.104227(1) atomic units (without the mass-polarization correction), has been obtained.

  14. Pierre Gorce working on a helium pump.

    CERN Multimedia

    1975-01-01

    This type of pump was designed by Mario Morpurgo, to circulate liquid helium in superconducting magnets wound with hollow conductors. M. Morpurgo, Design and construction of a pump for liquid helium, CRYIOGENICS, February 1977, p. 91

  15. Helium release during shale deformation: Experimental validation

    Science.gov (United States)

    Bauer, Stephen J.; Gardner, W. Payton; Heath, Jason E.

    2016-07-01

    This work describes initial experimental results of helium tracer release monitoring during deformation of shale. Naturally occurring radiogenic 4He is present in high concentration in most shales. During rock deformation, accumulated helium could be released as fractures are created and new transport pathways are created. We present the results of an experimental study in which confined reservoir shale samples, cored parallel and perpendicular to bedding, which were initially saturated with helium to simulate reservoir conditions, are subjected to triaxial compressive deformation. During the deformation experiment, differential stress, axial, and radial strains are systematically tracked. Release of helium is dynamically measured using a helium mass spectrometer leak detector. Helium released during deformation is observable at the laboratory scale and the release is tightly coupled to the shale deformation. These first measurements of dynamic helium release from rocks undergoing deformation show that helium provides information on the evolution of microstructure as a function of changes in stress and strain.

  16. The cosmic production of Helium

    CERN Document Server

    Jiménez, R; MacDonald, J; Gibson, B K; Jimenez, Raul; Flynn, Chris; Donald, James Mac; Gibson, Brad K.

    2003-01-01

    We estimate the cosmic production rate of helium relative to metals ($\\Delta Y/\\Delta Z$) using K dwarf stars in the Hipparcos catalog with accurate spectroscopic metallicities. The best fitting value is $\\Delta Y/\\Delta Z=2.1 \\pm 0.4$ at the 68% confidence level. Our derived value agrees with determinations from HII regions and with theoretical predictions from stellar yields with standard assumptions for the initial mass function. The amount of helium in stars determines how long they live and therefore how fast they will enrich the insterstellar medium with fresh material.

  17. Negative ions in liquid helium

    Science.gov (United States)

    Khrapak, A. G.; Schmidt, W. F.

    2011-05-01

    The structure of negative ions in liquid 4He is analyzed. The possibility of cluster or bubble formation around impurity ions of both signs is discussed. It is shown that in superfluid helium, bubbles form around negative alkaline earth metal ions and clusters form around halogen ions. The nature of "fast" and "exotic" negative ions is also discussed. It is assumed that "fast" ions are negative ions of helium excimer molecules localized inside bubbles. "Exotic" ions are stable negative impurity ions, which are always present in small amounts in gas discharge plasmas. Bubbles or clusters with radii smaller the radius of electron bubbles develop around these ions.

  18. Membrane pumping technology, helium and hydrogen isotopes separation in the fusion hydrogen

    Energy Technology Data Exchange (ETDEWEB)

    Pigarov, A.Yu.; Pistunovich, V.I. [NFI RRC-Kurchatov Institute, Moscow (Russian Federation); Busnyuk, A.O. [Bonch-Bruyevich Electrotechnical Inst. of Communications, St. Petersburg (Russian Federation)] [and others

    1994-12-31

    A gas pumping system for the ITER, improved by implementation of superpermeable membranes for selective hydrogen isotope exhaust, is considered. The study of the pumping capability of a niobium membrane for a hydrogen-helium mixture has been fulfilled. The membrane superpermeability can be only realized for atomic hydrogen. Helium does not pass through the membrane, and its presence does not affect the hydrogen pumping. A detailed Monte Carlo simulation of gas behavior for the experimental facility has been done. The probability of permeation for a hydrogen atom for one collision with the membrane is {approximately}0.1; the same probability of molecule permeation is {approximately}10{sup {minus}5}. The probability for atomization, i.e. re-emission of an atomizer is {approximately}0.2; the probability of recombination of an atom is {approximately}0.2.

  19. A molecular dynamics simulation study of temperature and depth effect on helium bubble releasing from Ti surface

    Energy Technology Data Exchange (ETDEWEB)

    Liang, Li; Ma, Mingwang; Xiang, Wei; Wang, Yuan; Cheng, Yanlin; Tan, Xiaohua, E-mail: caepiee@163.com

    2015-10-05

    Highlights: • Features of helium bubble at varied depths in Ti are researched by MD simulation. • Effect of Temperature on helium bubble in Ti is researched by MD simulation. • The mechanism of helium bubble releasing from metal is clarified. - Abstract: Using molecular dynamics simulation, the effect of environment temperature and depth of helium bubble on its volume, pressure and releasing process in metal Ti is researched. First, through studying the statuses of helium bubble at different depths at 300 K, the regularity of helium bubble shape, volume and pressure is acquired. The results show that with depth augmenting, the pressure increases gradually, while the volume decreases, but these two parameters keep around some level when depth is greater than 2.6 nm. Then, the evolution of model system with helium bubble at various temperatures is simulated. On the whole, the critical releasing temperature increases with depth. Finally, the mechanism of helium bubble releasing from Ti surface is explained. It is found that the bubble would tear the Ti film above it when its pressure is greater than the tensile strength of metal film, and then helium atoms will release from the metal.

  20. Electron correlation dynamics of strong-field double ionization of atoms below recollision threshold

    Energy Technology Data Exchange (ETDEWEB)

    Liu Yunquan; Gong Qihuang [Department of Physics and State Key Laboratory for Mesoscopic Physics, Peking University, Beijing 100871 (China); Ye Difa; Liu Jie [Center for Applied Physics and Technology, Peking University, 100084 Beijing (China); Rudenko, A; Tschuch, S; Duerr, M; Moshammer, R; Ullrich, J [Max-Planck-Institut fuer Kernphysik, D-69117 Heidelberg (Germany); Siegel, M; Morgner, U, E-mail: yunquan.liu@pku.edu.cn [Leibniz Universitaet Hannover, Welfengarten 1, D-30167 Hannover (Germany)

    2011-02-01

    In recent combined experimental and theoretical study we have explored nonsequential double ionization of neon and argon atoms in the infrared light field (800nm) below the recollision threshold. We find that the two-electron correlation dynamics depends on atomic structure- 'side-by-side emission' (correlation) for Ne and 'back-to-back emission' (anticorrelation) for argon atoms. This can be explained theoretically within our three dimensional classical model calculation including tunnelling effect. The multiple recollisions as well as recollision-induced-excitation-tunnelling (RIET) effect dominate the anticorrelation of argon, whereas the laser-assisted instantaneous recollision dominates the correlation of neon.

  1. Helium in atmospheres of binary stars

    Energy Technology Data Exchange (ETDEWEB)

    Leushin, V.V. (Rostovskij-na-Donu Gosudarstvennyj Univ. (USSR). Nauchno-Issledovatel' skij Inst. Fiziki)

    The helium abundances were obtained for 25 bright components of binary stars by model atmosphere analysis. The helium abundance for binary stars that lie on the main sequence are larger in the average than in single normal stars. The stars on the Hertzsppung - russel diagram lie at a larger distance from the zero age line than those with normal helium abundance.

  2. The influence of neon or argon impurities on deuterium permeation in tungsten

    Energy Technology Data Exchange (ETDEWEB)

    Ishida, M., E-mail: ishida@st.eie.eng.osaka-u.ac.jp; Lee, H.T.; Ueda, Y.

    2015-08-15

    Nitrogen (N) or neon (Ne) in the divertor and argon (Ar) puffing in the first wall have been proposed to reduce the local power loads on tungsten (W) plasma facing components. The impurities sputter and modify the W surface, which can affect hydrogen (H, D, T) transport in W. In this study, mixed D + Ne or D + Ar ion driven permeation experiments were performed to investigate the influence of Ne or Ar impurities on D transport. The D permeation flux for mixed irradiation was lower in comparison to D-only irradiation at T > 500 K, opposite to trends observed for N. The reason for the observed decrease in permeation flux was interpreted to arise from combined effects of sputtering and possible precipitation. The lag times for D + Ne case was slower than D-only case, while D + Ar was faster. This indicates Ne precipitation effects may influence the H transport in W similar to helium.

  3. Nucleation and growth of helium bubbles in aluminum between 20 and 900 K

    DEFF Research Database (Denmark)

    Rajainmäki, H.; Linderoth, Søren; Hansen, H. E.

    1988-01-01

    The nucleation and growth of helium bubbles have been monitored in 3implanted aluminum by the positron-lifetime technique and transmission electron microscopy. Helium atoms are mobile during the implantation and are subsequently trapped by vacancies. The annealing stages I and III are observed...... at 40 and 200 K, respectively, in agreement with previous positron annihilation and electrical-resistivity data. The low implantation temperature of 20 K hinders bubble formation during implantation, but during isochronal annealing, around 425 K, helium starts to nucleate into bubbles via substitutional...... migration of the He-vacancy pairs. The migration energy for a He-vacancy pair is estimated to be 1.3±0.1 eV. Above 600 K the He bubbles grow through condensation of thermally produced vacancies, as well as bubble migration and coalescence. The created helium bubbles are extremely stable and survive...

  4. Argon gas flow through glass nanopipette

    Science.gov (United States)

    Takami, Tomohide; Nishimoto, Kiwamu; Goto, Tadahiko; Ogawa, Shuichi; Iwata, Futoshi; Takakuwa, Yuji

    2016-12-01

    We have observed the flow of argon gas through a glass nanopipette in vacuum. A glass nanopipette with an inner diameter of 100 nm and a shank length of 3 mm was set between vacuum chambers, and argon gas was introduced from the top of the nanopipette to the bottom. The exit pressure was monitored with an increase in entrance pressure in the range of 50-170 kPa. Knudsen flow was observed at an entrance pressure lower than 100 kPa, and Poiseuille flow was observed at an entrance pressure higher than 120 kPa. The proposed pressure-dependent gas flow method provides a means of evaluating the glass nanopipette before using it for various applications including nanodeposition to surfaces and femtoinjection to living cells.

  5. Abnormal epidermal changes after argon laser treatment

    Energy Technology Data Exchange (ETDEWEB)

    Neumann, R.A.; Knobler, R.M.; Aberer, E.; Klein, W.; Kocsis, F.; Ott, E. (Univ. of Vienna (Austria))

    1991-02-01

    A 26-year-old woman with a congenital port-wine stain on the forehead was treated three times at 2-month intervals with an argon laser. Six months after the last treatment, moderate blanching and mild scaling confined to the treated area was observed. A biopsy specimen of the treated area revealed a significant decrease in ectatic vessels. However, epidermal changes similar to those of actinic keratosis with disorganized cell layers and marked cytologic abnormalities were seen. Analysis of peripheral blood lymphocytes for a defect in DNA repair was negative. Multiple, argon laser-induced photothermal effects may be responsible for the changes observed in our case and may lead to premalignant epidermal transformation.

  6. Calibration of liquid argon and neon detectors with $^{83}Kr^m$

    CERN Document Server

    Lippincott, W H; Gastler, D; Kastens, L W; Kearns, E; McKinsey, D N; Nikkel, J A

    2009-01-01

    We report results from tests of $^{83}$Kr$^{\\mathrm{m}}$, as a calibration source in liquid argon and liquid neon. $^{83}$Kr$^{\\mathrm{m}}$ atoms are produced in the decay of $^{83}$Rb, and a clear $^{83}$Kr$^{\\mathrm{m}}$ scintillation peak at 41.5 keV appears in both liquids when filling our detector through a piece of zeolite coated with $^{83}$Rb. Based on this scintillation peak, we observe 6.0 photoelectrons/keV in liquid argon with a resolution of 6% ($\\sigma$/E) and 3.0 photoelectrons/keV in liquid neon with a resolution of 19% ($\\sigma$/E). The observed peak intensity subsequently decays with the $^{83}$Kr$^{\\mathrm{m}}$ half-life after stopping the fill, and we find evidence that the spatial location of $^{83}$Kr$^{\\mathrm{m}}$ atoms in the chamber can be resolved. $^{83}$Kr$^{\\mathrm{m}}$ will be a useful calibration source for liquid argon and neon dark matter and solar neutrino detectors.

  7. LIQUID ARGON CALORIMETER PERFORMANCE AT HIGH RATES

    CERN Document Server

    Kukhtin, V; The ATLAS collaboration

    2011-01-01

    The performance of the ATLAS liquid argon endcap and forward calorimeters has been projected at the planned high luminosity LHC option HL-LHC by exposing small calorimeter modules of the electromagnetic, hadronic, and forward calorimeters to high intensity proton beams at IHEP/Protvino accelerator. The results of HV current and of pulse shape analysis, and also the dependence of signal amplitude on beam intensity are presented.

  8. An impact hypothesis for Venus argon anomalies

    Science.gov (United States)

    Kaula, W. M.; Newman, W. I.

    1997-03-01

    The Ar-36+38 argon-excess anomally of Venus has been hypothesized to have its origin in the impact of an outer solar system body of about 100-km diameter. A critical evaluation is made of this hypothesis and its competitors; it is judged that its status must for the time being remain one of 'Sherlock Holmes' type, in that something so improbable must be accepted when all alternatives are eliminated.

  9. Helium resources of Mare Tranquillitatis

    Science.gov (United States)

    Cameron, Eugene N.

    Wisconsin Center for Space Automation and Robotics, Univ. of Wisc., Madison, Wisc. Mare Tranquillitatis, about 300000 sq km in area, is currently the most promising lunar source of He-3 for fueling fusion power plants on Earth. About 60 pct. of the mare regolith consists of particles 100 microns or less in diameter. Helium and other gases derived from the solar wind are concentrated in the fine size fractions. Studies of very small craters indicate that the average regolith exceeds 3 m in areas away from larger craters and other mare features not amenable to mining. There is no evidence of decrease of helium content of regolith and depth. Helium is known to be enriched in regoliths that are high in TiO2 content. Remote sensing indicates that about 90 pct. of Mare Tranquillitatis is covered by regolith ranging from about 6 to +7.5 pct. TiO2; inferred He contents range from 20 to at least 45 wppm total helium (7 to 18 wppb He-3). Detailed studies of craters and inferred ejecta halos displayed on high resolution photographs of the Apollo 11 and Ranger 8 areas suggest that as much as 50 pct. of the mare regolith may be physically minable, on average, with appropriate mining equipment. Assuming that the average thickness of regolith is 3 m, and that 50 pct. of the mare area is minable, the He-3 content of minable regolith containing 20 to 45 wppm total He is estimated at about 94,000 tonnes.

  10. Atomic hydrogen storage method and apparatus

    Science.gov (United States)

    Woollam, J. A. (Inventor)

    1980-01-01

    Atomic hydrogen, for use as a fuel or as an explosive, is stored in the presence of a strong magnetic field in exfoliated layered compounds such as molybdenum disulfide or an elemental layer material such as graphite. The compounds maintained at liquid helium temperatures and the atomic hydrogen is collected on the surfaces of the layered compound which are exposed during delamination (exfoliation). The strong magnetic field and the low temperature combine to prevent the atoms of hydrogen from recombining to form molecules.

  11. Torsional Alfven waves in solar partially ionized plasma: effects of neutral helium and stratification

    CERN Document Server

    Zaqarashvili, T V; Soler, R

    2012-01-01

    Ion-neutral collisions may lead to the damping of Alfven waves in chromospheric and prominence plasmas. Neutral helium atoms enhance the damping in certain temperature interval, where the ratio of neutral helium and neutral hydrogen atoms is increased. Therefore, the height-dependence of ionization degrees of hydrogen and helium may influence the damping rate of Alfven waves. We aim to study the effect of neutral helium in the damping of Alfven waves in stratified partially ionized plasma of the solar chromosphere. We consider a magnetic flux tube, which is expanded up to 1000 km height and then becomes vertical due to merging with neighboring tubes, and study the dynamics of linear torsional Alfven waves in the presence of neutral hydrogen and neutral helium atoms. We start with three-fluid description of plasma and consequently derive single-fluid magnetohydrodynamic (MHD) equations for torsional Alfven waves. Thin flux tube approximation allows to obtain the dispersion relation of the waves in the lower pa...

  12. Simplicity works for superfluid helium

    Energy Technology Data Exchange (ETDEWEB)

    Bowley, Roger [University of Nottingham, Nottingham (United Kingdom)

    2000-02-01

    The famous philosopher Karl Popper once said that ''science is the art of systematic oversimplification''. Indeed, when faced with a new puzzle the trick is to simplify it without losing the essential physics - something that is easier said than done. However, this approach has paid off recently in low-temperature physics. Last year Richard Packard, Seamus Davis and co-workers at the University of California at Berkeley encountered a puzzling new phenomenon in superfluid helium-3, a quantum fluid that remains a liquid close to absolute zero and exhibits unusual properties such as the ability to flow without friction (A Machenkov et al. 1999 Phys. Rev. Lett. 83 3860). Previous experiments had revealed that certain effects in liquid helium are analogous to effects observed in superconductors, materials that lose all resistance to electric current at low temperatures. When the Berkeley researchers connected two reservoirs of superfluid helium-3, the superfluid flowed back and forth through apertures that formed a ''weak link'' between the two containers. This behaviour is similar to the oscillatory current of electrons that can flow across an insulating gap separating two superconductors - a device that is known as a Josephson junction. What was puzzling about the Berkeley results was that the helium-3 had two different stable configurations, both of which behaved in an unconventional way compared with a Josephson junction. This puzzle has now been solved independently by Sidney Yip at the National Center for Theoretical Sciences in Taiwan, and by Janne Viljas and Erkki Thuneberg at the Helsinki University of Technology in Finland (Phys. Rev. Lett. 1999 83 3864 and 3868). In this article the author describes the latest research on superfluid helium. (UK)

  13. Novel Diamond Films Synthesis Strategy: Methanol and Argon Atmosphere by Microwave Plasma CVD Method Without Hydrogen

    Science.gov (United States)

    Yang, Li; Jiang, Caiyi; Guo, Shenghui; Zhang, Libo; Gao, Jiyun; Peng, Jinhui; Hu, Tu; Wang, Liang

    2016-09-01

    Diamond thin films are grown on silicon substrates by only using methanol and argon mixtures in microwave plasma chemical vapor deposition (MPCVD) reactor. It is worth mentioning that the novel strategy makes the synthesis reaction works smoothly without hydrogen atmosphere, and the substrates temperature is only 500 °C. The evidence of surface morphology and thickness under different time is obtained by characterizing the samples using scanning electron microscopy (SEM). X-ray diffractometer (XRD) spectrum reveals that the preferential orientation of (111) plane sample is obtained. The Raman spectra indicate that the dominant component of all the samples is a diamond. Moreover, the diamond phase content of the targeted films was quantitatively analyzed by X-ray photoelectron spectroscopy (XPS) method, and the surface roughness of diamond films was investigated by atomic force microscope (AFM). Meanwhile, the possible synthesis mechanism of the diamond films in methanol- and argon-mixed atmosphere was discussed.

  14. Characteristics of a DC discharge with a water cathode in argon

    Energy Technology Data Exchange (ETDEWEB)

    Smirnov, S. A.; Shutov, D. A.; Bobkova, E. S.; Rybkin, V. V., E-mail: rybkin@isuct.ru [Ivanovo State University of Chemistry and Technology (Russian Federation)

    2016-01-15

    The characteristics of a dc discharge excited between a metal anode and a water cathode in argon were studied experimentally. The dimensions of the positive column and the electric field in it were measured, and the vibrational temperature in the positive column was determined from the N{sub 2}C{sup 3}Π{sub u} → B{sup 3}Π{sub g} (0–2) emission band. It is shown that the power deposited in the positive column is almost entirely spent on gas heating. The obtained dependence of the reduced electric field on the gas pressure and the ionization frequencies calculated by solving the Boltzmann equation indicate that electrons are lost diffusively, whereas ionization proceeds in a stepwise manner via the lower metastable states of argon atoms.

  15. Influence of dissociative recombination on the LTE of argon high-frequency plasmas at atmospheric pressure

    CERN Document Server

    Sainz, A; García, M C; Calzada, M D; Sainz, Abel; Margot, Joelle; Garcia, Maria Carmen; Calzada, Maria Dolores

    2004-01-01

    This work presents a few preliminary results from a collisional-radiative (CR) model intended to describe an argon microwave (2.45 GHz) plasma at atmospheric pressure. This model aims to investigate the influence of dissociative recombination products on the Saha-Boltzmann plasma equilibrium. The model is tested through comparison with experimental results obtained in an argon plasma column generated by a traveling electromagnetic surface-wave, which is suitable to perform a parametric investigation of the plasma. It is shown that dissociative recombination predominantly populates the 4s levels and the ground state. It is further observed that it strongly influences the population of the levels, specially those of lower energy. However, the higher levels (close to the ionization limit) appear to be in equilibrium whatever the plasma density. This allows assuming that the excitation temperature Texc determined from the upper levels in the atomic system in the Boltzmann-plot is equal to Te.

  16. Nanometer-scale sharpening and surface roughening of ZnO nanorods by argon ion bombardment

    Energy Technology Data Exchange (ETDEWEB)

    Chatterjee, Shyamal, E-mail: shyamal@iitbbs.ac.in [School of Basic Sciences, Indian Institute of Technology, Bhubaneswar 751013 (India); Behera, Akshaya K. [School of Basic Sciences, Indian Institute of Technology, Bhubaneswar 751013 (India); Banerjee, Amarabha; Tribedi, Lokesh C. [Tata Institute of Fundamental Research, Homi Bhabha Road, Mumbai 400005 (India); Som, Tapobrata [Institute of Physics, Sachivalaya Marg, Bhubaneswar 751005 (India); Ayyub, Pushan, E-mail: pushan@tifr.res.in [Tata Institute of Fundamental Research, Homi Bhabha Road, Mumbai 400005 (India)

    2012-07-01

    We report the effects of exposing a hydrothermally grown, single crystalline ZnO nanorod array to a beam of 50 keV argon ions at room temperature. High resolution electron microscopy reveals that the ion bombardment results in a nanometer-scale roughening of the nanorod sidewalls, which were almost atomically flat in the pristine sample. Ion bombardment further causes the flat, Almost-Equal-To 100 nm diameter nanorod tips to get sharpened to ultrafine points less than 10 nm across. While tip sharpening is attributed to preferential sputtering, the formation of crystalline surface protuberances can be ascribed to surface instability due to curvature dependent sputtering and surface diffusion under argon-ion bombardment. Both the nanoscale roughening as well as the tip sharpening are expected to favorably impact a wide variety of applications, such as those involving catalysis, gas sensing, solar cells, field emission and gas discharge.

  17. Photochemistry of the ozone-water complex in cryogenic neon, argon, and krypton matrixes.

    Science.gov (United States)

    Tsuge, Masashi; Tsuji, Kazuhide; Kawai, Akio; Shibuya, Kazuhiko

    2013-12-12

    The photochemistry of ozone-water complexes and the wavelength dependence of the reactions were studied by matrix isolation FTIR spectrometry in neon, argon, and krypton matrixes. Hydrogen peroxide was formed upon the irradiation of UV light below 355 nm. Quantitative analyses of the reactant and product were performed to evaluate the matrix cage effect of the photoreaction. In argon and krypton matrixes, a bimolecular O((1)D) + H2O → H2O2 reaction was found to occur to form hydrogen peroxide, where the O((1)D) atom generated by the photolysis of ozone diffused in the cryogenic solids to encounter water. In a neon matrix, hydrogen peroxide was generated through intracage photoreaction of the ozone-water complex, indicating that a neon matrix medium is most appropriate to study the photochemistry of the ozone-water complex.

  18. The primordial helium abundance from updated emissivities

    Energy Technology Data Exchange (ETDEWEB)

    Aver, Erik [Department of Physics, Gonzaga University, 502 E Boone Ave, Spokane, WA, 99258 (United States); Olive, Keith A.; Skillman, Evan D. [School of Physics and Astronomy, University of Minnesota, 116 Church St. SE, Minneapolis, MN, 55455 (United States); Porter, R.L., E-mail: aver@gonzaga.edu, E-mail: olive@umn.edu, E-mail: ryanlporter@gmail.com, E-mail: skillman@astro.umn.edu [Department of Physics and Astronomy, University of Georgia, Athens, GA, 30602 (United States)

    2013-11-01

    Observations of metal-poor extragalactic H II regions allow the determination of the primordial helium abundance, Y{sub p}. The He I emissivities are the foundation of the model of the H II region's emission. Porter, Ferland, Storey, and Detisch (2012) have recently published updated He I emissivities based on improved photoionization cross-sections. We incorporate these new atomic data and update our recent Markov Chain Monte Carlo analysis of the dataset published by Izotov, Thuan, and Stasi'nska (2007). As before, cuts are made to promote quality and reliability, and only solutions which fit the data within 95% confidence level are used to determine the primordial He abundance. The previously qualifying dataset is almost entirely retained and with strong concordance between the physical parameters. Overall, an upward bias from the new emissivities leads to a decrease in Y{sub p}. In addition, we find a general trend to larger uncertainties in individual objects (due to changes in the emissivities) and an increased variance (due to additional objects included). From a regression to zero metallicity, we determine Y{sub p} = 0.2465 ± 0.0097, in good agreement with the BBN result, Y{sub p} = 0.2485 ± 0.0002, based on the Planck determination of the baryon density. In the future, a better understanding of why a large fraction of spectra are not well fit by the model will be crucial to achieving an increase in the precision of the primordial helium abundance determination.

  19. Electrical breakdown in helium cells at low temperature

    Science.gov (United States)

    Sethumadhavan, Bhaskar

    2007-05-01

    We have encountered a new phenomenon in the development of a prototype detector of solar neutrinos using liquid helium in which recoil electrons from neutrino scattering are to be detected by extracting them from the liquid and accelerating them in the vacuum by an electric field. In order to understand the possible constraints on such a particle detector using superfluid helium, we have studied the currents produced by a radioactive source in a helium cell having a liquid/vacuum interface at 100 mK. A number of phenomena have been observed that have not been described in the literature. These include the following. (1) The current at very low voltages, V ˜ 0, in a cell having a free surface can be up to 100 times greater than in a filled cell. (2) There is a large amplification of current in modest electric fields with a free surface present in the cell. (3) The amplification becomes sufficiently large such that a breakdown occurs at potential differences across the vacuum on the order of 1000 V. The results for a partially filled cell can be understood in terms of Penning ionization of excimers on the surface of the helium and the subsequent acceleration of electrons across the vacuum. Triplet excimers are created in the liquid by the radioactive source. These excimers propagate with a mean free path that is determined by scattering from 3He atoms and quasiparticles in the superfluid He. If an excimer reaches the surface, it is bound there but is free to move in the plane of the surface. Once bound to the surface these mobile excimers become distributed uniformly over all surfaces (bulk liquid and the film). They move about and annihilate in pairs through the Penning ionization process to create electrons and positive helium ions in the vacuum. An electron in the vacuum in the presence of an electric field is always destined to hit liquid helium, either the bulk liquid or the film on the top surface of the cell. If the energy of the electron is sufficient to

  20. Effects of argon ion irradiation on nucleation and growth of silver nanoparticles in a soda-glass matrix

    Directory of Open Access Journals (Sweden)

    P. Gangopadhyay

    2011-09-01

    Full Text Available The present article explores an experimental study for nucleation and non-equilibrium growth of silver nanoparticles in a soda-glass matrix. Ion-irradiation induced recoiling of silver atoms with argon ions (at energy 100 keV facilitates nucleation as well as growth of the silver nanoparticles in the soda-glass matrix. Small growth of the silver nanoparticles in the soda-glass matrix has been experimentally observed after the irradiation with higher fluences of the argon ions. Role of the argon ions for the evolution of the silver nanoparticles in the soda-glass matrix has been elucidated in the present report. With increase of the argon-ion fluences, while slight athermal growth of the silver nanoparticles has been estimated, drastic increase in the optical responses and Rutherford backscattering (RBS yields of the silver nanoparticles have been observed in the sample with the maximum fluences. Possible correlations of increase of argon-ion fluences and the observed experimental results (optical and RBS, in particular have been explained in this article. Although it has been demonstrated using the silver metal film on a soda-glass substrate as a model example, the non-equilibrium approach of nucleation and ion-beam controlled growth of metal nanoparticles in a matrix should be applicable to other immiscible systems as well.