Particle emissions from compressed natural gas engines

International Nuclear Information System (INIS)

Ristovski, Z.D.; Morawska, L.; Hitchins, J.; Thomas, S.; Greenaway, C.; Gilbert, D.

2000-01-01

This paper presents the results of measurements conducted to determine particle and gas emissions from two large compressed natural gas (CNG) spark ignition (SI) engines. Particle size distributions in the range from 0.01-30 μm, and gas composition were measured for five power settings of the engines: 35, 50, 65, 80 and 100% of full power. Particle emissions in the size range between 0.5 and 30 μm, measured by the aerodynamic particle sizer (APS), were very low at a level below two particles cm -3 . These concentrations were comparable with average ambient concentration, and were not considered in the succeeding analysis. Both engines produce significant amounts of particles in the size range between 0.015 and 0.7 μm, measured by the scanning mobility particle size (SMPS). Maximum number of concentrations of about 1 x 10 7 particles cm -3 were very similar for both engines. The CMDs were in the range between 0.020 and 0.060 μm. The observed levels of particulate emission are in terms of number of the same order as emissions from heavy duty diesel engines (Morawska et al., Environ. Sci. Tech. 32, 2033-2042). On the other hand, emissions of CO and NO x of 5.53 and 3.33 g k W h -1 , respectively, for one of the tested engines, were considerably lower than set by the standards. According to the specifications for the gas emissions, provided by the US EPA (US EPA, 1997), this engine can be considered as a 'low-emission' engine, although emissions of submicrometer particles are of the same order as heavy-duty vehicles. (Author)

The fine particle emissions of energy production in Finland

International Nuclear Information System (INIS)

Ohlstroem, M.

1998-01-01

The main purpose of this master's thesis was to define the fine particle (PM2.5, diameter under 2,5 μm) emissions of the energy production and to compare the calculated emission factors between different energy production concepts. The purpose was also to define what is known about fine particle emissions and what should still be studied/measured. The purpose was also to compare briefly the fine particle emissions of energy production and vehicle traffic, and their correlations to the fine particle concentrations of urban air. In the theory part of this work a literature survey was made about fine particles in energy production, especially how they form and how they are separated from the flue gas. In addition, the health effects caused by fine particles, and different measuring instruments were presented briefly. In the experimental part of this work, the aim was to find out the fine particle emissions of different energy production processes by calculating specific emission factors (mg/MJ fuel ) from powerplants' annual total particulate matter emissions (t/a), which were obtained from VAHTI-database system maintained by the Finnish Environmental Institute, and by evaluating the share of fine particles from total emissions with the help of existing measurement results. Only those energy production processes which produce significantly direct emissions of solid particles have been treated (pulverised combustion and oil burners from burner combustion, fluidized bed combustion processes, grate boilers, recovery boilers and diesel engines). The processes have been classified according to boiler type, size category, main fuel and also according to dust separation devices. To be able to compare different energy production processes, shared specific emission factor have been calculated for the similar subprocesses. The fine particle emissions depend strongest on the boiler size category and dust separation devices used. Spent fuel or combustion technique does not have

Personal recollections of the discovery of fast particles

International Nuclear Information System (INIS)

Walton, E.T.S.

1984-01-01

The author gives an account of the Cavendish Laboratory in Cambridge, and its staff, in the late 1920's when he arrived there as a research student. His chosen line of research was to produce fast particles (faster than the natural alpha particles then available) which could be used to bombard atoms to produce disintegration. He recounts how he developed, with J.D. Cockcroft, a linear method of accelerating particles by the direct application of high voltage. A picture of the Cockcroft-Walton accelerator of 1932 is shown. In this a proton beam bombarded a lithium target and two fast alpha particles were emitted, travelling in opposite directions. (UK)

Particle number emissions of gasoline hybrid electric vehicles; Partikelanzahl-Emission bei Hybridfahrzeugen mit Ottomotor

Energy Technology Data Exchange (ETDEWEB)

Porter, Scott [Horiba Instruments Inc., Ann Arbor, MI (United States)

2012-04-15

Hybrid Electric Vehicles (HEV) are commonly reputed to be environmentally friendly. Different studies show that this assumption raises some questions in terms of particle number emissions. Against the background that upcoming emission standards will not only limit particle matter emissions but also particle number emissions for gasoline engines, the exhaust behaviour of downsized gasoline engines used in HEV should be investigated more extensively. A Horiba study compares the particle number emissions of a gasoline vehicle to those of a gasoline powered HEV. (orig.)

Particle Emissions from Domestic Gas Cookers

DEFF Research Database (Denmark)

Glarborg, Peter; Livbjerg, Hans; Wagner, Ayten Yilmaz

2010-01-01

The authors experimentally studied the formation of submicron particles from a domestic gas cooker in a compartment free from external particle sources. The effects of fuel (methane, natural gas, odorant-free natural gas), primary aeration, flow rate, and fuel sulphur content on particle emissions...... of the emitted particles were found to have a mean value of about 7 nm for partially premixed flames, increasing to ∼10 nm for nonpremixed flames. The quantity of primary air had a strong impact on the particle emissions, showing a minimum at a primary aeration level of 60-65%. Presence of sulphur in small...... quantities may enhance particle formation under some conditions, but results were not conclusive....

Airborne emission measurements of SO2 , NOx and particles from individual ships using a sniffer technique

Science.gov (United States)

Beecken, J.; Mellqvist, J.; Salo, K.; Ekholm, J.; Jalkanen, J.-P.

2014-07-01

A dedicated system for airborne ship emission measurements of SO2, NOx and particles has been developed and used from several small aircraft. The system has been adapted for fast response measurements at 1 Hz, and the use of several of the instruments is unique. The uncertainty of the given data is about 20% for SO2 and 24% for NOx emission factors. The mean values with one standard deviation for multiple measurements of 158 ships measured from the air on the Baltic and North Sea during 2011 and 2012 show emission factors of 18.8 ± 6.5 g kg-1 fuel , 66.6 ± 23.4 g kg-1 fuel and 1.8 ± 1.3 1016 particles kg-1 fuel for SO2, NOx and particle number, respectively. The particle size distributions were measured for particle diameters between 15 and 560 nm. The mean sizes of the particles are between 45 and 54 nm dependent on the distance to the source, and the number size distribution is monomodal. Concerning the sulfur fuel content, around 85% of the monitored ships comply with the International Maritime Organization (IMO) limits. The reduction of the sulfur emission control area (SECA) limit from 1.5 to 1% in 2010 appears to have contributed to reduction of sulfur emissions that were measured in earlier studies from 2007 to 2009. The presented method can be implemented for regular ship compliance monitoring.

Pre-scission particle and gamma-ray emission in heavy-ion induced fission

International Nuclear Information System (INIS)

Newton, J.O.

1989-02-01

An introduction is given to the physics of the equilibrium transition model and of dissipative nuclear dynamics. Experimental data on pre-scission particle and gamma-ray emission and their interpretation are reviewed. They appear to indicate overdamped motion of the nuclear fluid. A time scale for compound-nucleus fission of about 30x10 -21 sec or greater is indicated, whilst that for quasi- or fast-fission is somewhat shorter. 99 refs., 28 figs

MONDO: A tracker for the characterization of secondary fast and ultrafast neutrons emitted in particle therapy

Science.gov (United States)

Mirabelli, R.; Battistoni, G.; Giacometti, V.; Patera, V.; Pinci, D.; Sarti, A.; Sciubba, A.; Traini, G.; Marafini, M.

2018-01-01

In Particle Therapy (PT) accelerated charged particles and light ions are used for treating tumors. One of the main limitation to the precision of PT is the emission of secondary particles due to the beam interaction with the patient: secondary emitted neutrons can release a significant dose far from the tumor. Therefore, a precise characterization of their flux, production energy and angle distribution is eagerly needed in order to improve the Treatment Planning Systems (TPS) codes. The principal aim of the MONDO (MOnitor for Neutron Dose in hadrOntherapy) project is the development of a tracking device optimized for the detection of fast and ultra-fast secondary neutrons emitted in PT. The detector consists of a matrix of scintillating square fibres coupled with a CMOS-based readout. Here, we present the characterization of the detector tracker prototype and CMOS-based digital SPAD (Single Photon Avalanche Diode) array sensor tested with protons at the Beam Test Facility (Frascati, Italy) and at the Proton Therapy Centre (Trento, Italy), respectively.

Stimulated-emission effects in particle creation near black holes

International Nuclear Information System (INIS)

Wald, R.M.

1976-01-01

It has recently been shown that if a black hole is formed by gravitational collapse, spontaneous particle creation will occur and a thermal spectrum of all species of particles will be emitted to infinity if the quantum matter was initially in the vacuum state. In this paper we investigate the stimulated-emission effects which occur if particles are present initially. We show in general that for a Hermitian scalar field in an external potential or in curved, asymptotically flat spacetime, stimulated-emission effects can occur precisely in those modes for which there is spontaneous particle creation from the vacuum. For the case of a Schwarzschild black hole, this result appears paradoxical, since spontaneous emission occurs at late times but there is no classical analog of stimulated emission at late times. The resolution of this paradox is that in order to induce emission of particles which emerge at late times one must send in particles at early times, so that they reach the black hole very near the instant of its formation. However, enormous energy is required of these incoming particles in order to stimulate emission of particles which emerge at late times. Thus, for a Schwarzschild black hole, even if particles are initially present (with limited energy) they will induce emission only at early times; at late times one will see only the spontaneously emitted blackbody thermal radiation. For the case of a Kerr black hole stimulated emission can be induced by particles sent in at late times with the appropriate frequencies and angular dependence. If the number of incoming particles is large, this quantum stimulated emission just gives the classical superradiant scattering

Composite-particle emission in the reaction p+Au at 2.5 GeV

Energy Technology Data Exchange (ETDEWEB)

Letourneau, A.; Bohm, A.; Galin, J.; Lott, B.; Peghaire, A. [Grand Accelerateur National d' Ions Lourds (GANIL), 14 - Caen (France); Enke, M.; Herbach, C.M.; Hilscher, D.; Jahnke, U.; Tishchenko, V. [Hahn Meitner Institute, Berlin (Germany); Filges, D.; Goldenbaum, F.; Neef, R.D.; Nunighoff, K.; Paul, N.; Sterzenbach, G. [Institut fur Kernphysik, Julich (Germany); Pienkowski, L. [Warsaw Universitaire, Heavy Ion Lab. (Poland); Toke, J.; Schroder, U. [Rochester, University, New York (United States)

2002-06-01

The emission of composite-particles is studied in the reaction p+Au at E{sub p} = 2.5 GeV, in addition to neutrons and protons. Most particle energy spectra feature an evaporation spectrum superimposed on an exponential high-energy, non-statistical component. Comparisons are first made with the predictions by a two-stage hybrid reaction model, where an intra-nuclear cascade (INC) simulation is followed by a statistical evaporation process. The high-energy proton component is identified as product of the fast pre-equilibrium INC, since it is rather well reproduced by the INCL2.0 intra-nuclear cascade calculations simulating the first reaction stage. The low-energy spectral components are well understood in terms of sequential particle evaporation from the hot nuclear target remnants of the fast INC. Evaporation is modeled using the statistical code GEMINI. Implementation of a simple coalescence model in the INC code can provide a reasonable description of the multiplicities of high-energy composite particles such as {sup 2-3}H and {sup 3}He. However, this is done at the expense of {sup 1}H which then fails to reproduce the experimental energy spectra. (authors)

Pre-equilibrium complex particle emission

International Nuclear Information System (INIS)

Bĕták, E.

2002-01-01

Semi-classical (phenomenological) pre-equilibrium emission of clusters of nucleons (complex particles) such as deuterons, tritons, helions and α particles from reactions induced by light projectiles (nucleons to α’s) is addressed. The main attention is given to the hard components in the emission energetic spectra, which play an increasing role at incident energies above 20 MeV, and are currently attributed to a presence of some kind of pre-equilibrium processes. In addition, the mechanisms of cluster reactions show special features such as the competition between pickup and knockout processes and the contributions of several successive steps in the reaction. The main frame used here to illustrate the processes and interplays of the competing mechanisms of pre-equilibrium cluster formation and emission, namely the coalescence, pick-up and knock-out, is the pre-equilibrium exciton model. It obviously contains the process of clusterization itself as its organic part. The most important case of complex particles with the largest amount of experimental data is that of alpha emission, which therefore naturally attracts most of the attention and where the widest range of possible mechanisms is available on the market. The loosely bound ejectiles, on the other side, are usually not able to demonstrate all features of the whole spectrum of contributing mechanisms, but they are nevertheless an important link between the nucleon emission and the cluster one.

Simulating Biomass Fast Pyrolysis at the Single Particle Scale

Energy Technology Data Exchange (ETDEWEB)

Ciesielski, Peter [National Renewable Energy Laboratory (NREL); Wiggins, Gavin [ORNL; Daw, C Stuart [ORNL; Jakes, Joseph E. [U.S. Forest Service, Forest Products Laboratory, Madison, Wisconsin, USA

2017-07-01

Simulating fast pyrolysis at the scale of single particles allows for the investigation of the impacts of feedstock-specific parameters such as particle size, shape, and species of origin. For this reason particle-scale modeling has emerged as an important tool for understanding how variations in feedstock properties affect the outcomes of pyrolysis processes. The origins of feedstock properties are largely dictated by the composition and hierarchical structure of biomass, from the microstructural porosity to the external morphology of milled particles. These properties may be accounted for in simulations of fast pyrolysis by several different computational approaches depending on the level of structural and chemical complexity included in the model. The predictive utility of particle-scale simulations of fast pyrolysis can still be enhanced substantially by advancements in several areas. Most notably, considerable progress would be facilitated by the development of pyrolysis kinetic schemes that are decoupled from transport phenomena, predict product evolution from whole-biomass with increased chemical speciation, and are still tractable with present-day computational resources.

Transient particle emission measurement with optical techniques

Science.gov (United States)

Bermúdez, Vicente; Luján, José M.; Serrano, José R.; Pla, Benjamín

2008-06-01

Particulate matter is responsible for some respiratory and cardiovascular diseases. In addition, it is one of the most important pollutants of high-speed direct injection (HSDI) passenger car engines. Current legislation requires particulate dilution tunnels for particulate matter measuring. However for development work, dilution tunnels are expensive and sometimes not useful since they are not able to quantify real-time particulate emissions during transient operation. In this study, the use of a continuous measurement opacimeter and a fast response HFID is proven to be a good alternative to obtain instantaneous particle mass emissions during transient operation (due to particulate matter consisting mainly of soot and SOF). Some methods and correlations available from literature, but developed for steady conditions, are evaluated during transient operation by comparing with mini-tunnel measurements during the entire MVEG-A transient cycle. A new correlation was also derived from this evaluation. Results for soot and SOF (obtained from the new correlation proposed) are compared with soot and SOF captured with particulate filters, which have been separated by means of an SOF extraction method. Finally, as an example of ECU design strategies using these sort of correlations, the EGR valve opening is optimized during transient operation. The optimization is performed while simultaneously taking into account instantaneous fuel consumption, particulate emissions (calculated with the proposed correlation) and other regulated engine pollutants.

Fast Particle Interaction With Waves In Fusion Plasmas

International Nuclear Information System (INIS)

Breizman, Boris

2006-01-01

There are two well-known motivations for theoretical studies of fast particle interaction with waves in magnetic confinement devices. One is the challenge of avoiding strong collective losses of alpha particles and beam ions in future burning plasma experiments. The other one is the compelling need to quantitatively interpret the large amount of experimental data from JET, TFTR, JT-60U, DIII-D, and other machines. Such interpretation involves unique diagnostic opportunities offered by MHD spectroscopy. This report discusses how the present theory responds to the stated challenges and what theoretical and computational advances are required to address the outstanding problems. More specifically, this paper deals with the following topics: predictive capabilities of linear theory and simulations; theory of Alfven cascades; diagnostic opportunities based on linear and nonlinear properties of unstable modes; interplay of kinetic and fluid nonlinearities; fast chirping phenomena for non-perturbative modes; and global transport of fast particles. Recent results are presented on some of the listed topics, although the main goal is to identify critical issues for future work

Signature of intermittent behavior in the emission spectra of target associated particles from 84Kr-AgBr interactions at 0.95 GeV/A

International Nuclear Information System (INIS)

Bhattacharjee, B.

2005-01-01

Intermittency and fractal behavior have been studied for emission spectra of target associated fast and slow particles from 84 Kr-AgBr interactions at 0.95 GeV/A. Intermittent behavior is observed for both knocked out and slow target fragments. In both the cases anomalous dimensions are seen to increase with the order of moments thereby indicating the association of multifractility with production mechanism of both fast and slow target associated particles

GAMMA-RAY EMISSION OF ACCELERATED PARTICLES ESCAPING A SUPERNOVA REMNANT IN A MOLECULAR CLOUD

International Nuclear Information System (INIS)

Ellison, Donald C.; Bykov, Andrei M.

2011-01-01

We present a model of gamma-ray emission from core-collapse supernovae (SNe) originating from the explosions of massive young stars. The fast forward shock of the supernova remnant (SNR) can accelerate particles by diffusive shock acceleration (DSA) in a cavern blown by a strong, pre-SN stellar wind. As a fundamental part of nonlinear DSA, some fraction of the accelerated particles escape the shock and interact with a surrounding massive dense shell producing hard photon emission. To calculate this emission, we have developed a new Monte Carlo technique for propagating the cosmic rays (CRs) produced by the forward shock of the SNR, into the dense, external material. This technique is incorporated in a hydrodynamic model of an evolving SNR which includes the nonlinear feedback of CRs on the SNR evolution, the production of escaping CRs along with those that remain trapped within the remnant, and the broadband emission of radiation from trapped and escaping CRs. While our combined CR-hydro-escape model is quite general and applies to both core collapse and thermonuclear SNe, the parameters we choose for our discussion here are more typical of SNRs from very massive stars whose emission spectra differ somewhat from those produced by lower mass progenitors directly interacting with a molecular cloud.

The practical model of electron emission in the radioisotope battery by fast ions

International Nuclear Information System (INIS)

Erokhine, N.S.; Balebanov, V.M.

2003-01-01

Under the theoretical analysis of secondary-emission radioisotope source of current the estimate of energy spectrum F(E) of secondary electrons with energy E emitted from films is the important problem. This characteristic knowledge allows, in particular, studying the volt-ampere function, the dependence of electric power deposited in the load on the system parameters and so on. Since the rigorous calculations of energy spectrum F(E) are the complicated enough and labour-intensive there is necessity to elaborate the practical model which allows by the simple computer routine on the basis of generalized data (both experimental measurements and theoretical calculations) on the stopping powers and mean free path of suprathermal electrons to perform reliable express-estimates of the energy spectrum F(E) and the volt-ampere function I(V) for the concrete materials of battery emitter films. This paper devoted to description of of the practical model to calculate electron emission characteristics under the passage of fast ion fluxes from the radioisotope source through the battery emitter. The analytical approximations for the stopping power of emitter materials, the electron inelastic mean free path, the ion production of fast electrons and the probability for them to arrive the film surface are taken into account. In the cases of copper and gold films, the secondary electron escaping depth, the position of energy spectrum peak are considered in the dependence on surface potential barrier magnitude U. According to our calculations the energy spectrum peak shifted to higher electron energy under the U growth. The model described may be used for express estimates and computer simulations of fast alpha-particles and suprathermal electrons interactions with the solid state plasma of battery emitter films, to study the electron emission layer characteristics including the secondary electron escaping depth, to find the optimum conditions for excitation of nonequilibrium

Determining size-specific emission factors for environmental tobacco smoke particles

Energy Technology Data Exchange (ETDEWEB)

Klepeis, Neil E.; Apte, Michael G.; Gundel, Lara A.; Sextro, Richard G.; Nazaroff, William W.

2002-07-07

Because size is a major controlling factor for indoor airborne particle behavior, human particle exposure assessments will benefit from improved knowledge of size-specific particle emissions. We report a method of inferring size-specific mass emission factors for indoor sources that makes use of an indoor aerosol dynamics model, measured particle concentration time series data, and an optimization routine. This approach provides--in addition to estimates of the emissions size distribution and integrated emission factors--estimates of deposition rate, an enhanced understanding of particle dynamics, and information about model performance. We applied the method to size-specific environmental tobacco smoke (ETS) particle concentrations measured every minute with an 8-channel optical particle counter (PMS-LASAIR; 0.1-2+ micrometer diameters) and every 10 or 30 min with a 34-channel differential mobility particle sizer (TSI-DMPS; 0.01-1+ micrometer diameters) after a single cigarette or cigar was machine-smoked inside a low air-exchange-rate 20 m{sup 3} chamber. The aerosol dynamics model provided good fits to observed concentrations when using optimized values of mass emission rate and deposition rate for each particle size range as input. Small discrepancies observed in the first 1-2 hours after smoking are likely due to the effect of particle evaporation, a process neglected by the model. Size-specific ETS particle emission factors were fit with log-normal distributions, yielding an average mass median diameter of 0.2 micrometers and an average geometric standard deviation of 2.3 with no systematic differences between cigars and cigarettes. The equivalent total particle emission rate, obtained integrating each size distribution, was 0.2-0.7 mg/min for cigars and 0.7-0.9 mg/min for cigarettes.

Emissions of soot particles from heat generators

Science.gov (United States)

Lyubov, V. K.; Popov, A. N.; Popova, E. I.

2017-11-01

«Soot carbon» or «Soot» - incomplete combustion or thermal decomposition particulate carbon product of hydrocarbons consisting of particles of various shapes and sizes. Soot particles are harmful substances Class 2 and like a dust dispersed by wind for thousands of kilometers. Soot have more powerful negative factor than carbon dioxide. Therefore, more strict requirements on ecological and economical performance for energy facilities at Arctic areas have to be developed to protect fragile Arctic ecosystems and global climate change from degradation and destruction. Quantity of soot particles in the flue gases of energy facilities is a criterion of effectiveness for organization of the burning process. Some of heat generators do not provide the required energy and environmental efficiency which results in irrational use of energy resources and acute pollution of environment. The paper summarizes the results of experimental study of solid particles emission from wide range of capacity boilers burning different organic fuels (natural gas, fuel oil, coal and biofuels). Special attention is paid to environmental and energy performance of the biofuels combustion. Emissions of soot particles PM2.5 are listed. Structure, composition and dimensions of entrained particles with the use of electronic scanning microscope Zeiss SIGMA VP were also studied. The results reveal an impact of several factors on soot particles emission.

Modeling of Particle Emission During Dry Orthogonal Cutting

Science.gov (United States)

Khettabi, Riad; Songmene, Victor; Zaghbani, Imed; Masounave, Jacques

2010-08-01

Because of the risks associated with exposure to metallic particles, efforts are being put into controlling and reducing them during the metal working process. Recent studies by the authors involved in this project have presented the effects of cutting speeds, workpiece material, and tool geometry on particle emission during dry machining; the authors have also proposed a new parameter, named the dust unit ( D u), for use in evaluating the quantity of particle emissions relative to the quantity of chips produced during a machining operation. In this study, a model for predicting the particle emission (dust unit) during orthogonal turning is proposed. This model, which is based on the energy approach combined with the microfriction and the plastic deformation of the material, takes into account the tool geometry, the properties of the worked material, the cutting conditions, and the chip segmentation. The model is validated using experimental results obtained during the orthogonal turning of 6061-T6 aluminum alloy, AISI 1018, AISI 4140 steels, and grey cast iron. A good agreement was found with experimental results. This model can help in designing strategies for reducing particle emission during machining processes, at the source.

Non-Maxwellian fast particle effects in gyrokinetic GENE simulations

Science.gov (United States)

Di Siena, A.; Görler, T.; Doerk, H.; Bilato, R.; Citrin, J.; Johnson, T.; Schneider, M.; Poli, E.; JET Contributors

2018-04-01

Fast ions have recently been found to significantly impact and partially suppress plasma turbulence both in experimental and numerical studies in a number of scenarios. Understanding the underlying physics and identifying the range of their beneficial effect is an essential task for future fusion reactors, where highly energetic ions are generated through fusion reactions and external heating schemes. However, in many of the gyrokinetic codes fast ions are, for simplicity, treated as equivalent-Maxwellian-distributed particle species, although it is well known that to rigorously model highly non-thermalised particles, a non-Maxwellian background distribution function is needed. To study the impact of this assumption, the gyrokinetic code GENE has recently been extended to support arbitrary background distribution functions which might be either analytical, e.g., slowing down and bi-Maxwellian, or obtained from numerical fast ion models. A particular JET plasma with strong fast-ion related turbulence suppression is revised with these new code capabilities both with linear and nonlinear gyrokinetic simulations. It appears that the fast ion stabilization tends to be less strong but still substantial with more realistic distributions, and this improves the quantitative power balance agreement with experiments.

Gaseous and particle emissions from an ethanol fumigated compression ignition engine

International Nuclear Information System (INIS)

Surawski, Nicholas C.; Ristovski, Zoran D.; Brown, Richard J.; Situ, Rong

2012-01-01

Highlights: ► Ethanol fumigation system fitted on a direct injection compression ignition engine. ► Ethanol substitutions up to 40% (by energy) were achieved. ► Gaseous and particle emissions were measured at intermediate speed. ► PM and NO emissions significantly reduced, whilst CO and HC increased. ► The number of particles emitted generally higher with ethanol fumigation. - Abstract: A 4-cylinder Ford 2701C test engine was used in this study to explore the impact of ethanol fumigation on gaseous and particle emission concentrations. The fumigation technique delivered vaporised ethanol into the intake manifold of the engine, using an injector, a pump and pressure regulator, a heat exchanger for vaporising ethanol and a separate fuel tank and lines. Gaseous (Nitric oxide (NO), Carbon monoxide (CO) and hydrocarbons (HC)) and particulate emissions (particle mass (PM 2.5 ) and particle number) testing was conducted at intermediate speed (1700 rpm) using 4 load settings with ethanol substitution percentages ranging from 10% to 40% (by energy). With ethanol fumigation, NO and PM 2.5 emissions were reduced, whereas CO and HC emissions increased considerably and particle number emissions increased at most test settings. It was found that ethanol fumigation reduced the excess air factor for the engine and this led to increased emissions of CO and HC, but decreased emissions of NO. PM 2.5 emissions were reduced with ethanol fumigation, as ethanol has a very low “sooting” tendency. This is due to the higher hydrogen-to-carbon ratio of this fuel, and also because ethanol does not contain aromatics, both of which are known soot precursors. The use of a diesel oxidation catalyst (as an after-treatment device) is recommended to achieve a reduction in the four pollutants that are currently regulated for compression ignition engines. The increase in particle number emissions with ethanol fumigation was due to the formation of volatile (organic) particles

Fast-ICCD photography and gated photon counting measurements of blackbody emission from particulates generated in the KrF-laser ablation of BN and YBCO

Energy Technology Data Exchange (ETDEWEB)

Geohegan, D.B.

1992-11-01

Fast intensified CCD photography and gated photon counting following KrF-laser irradiation of YBCO and BN targets reveals the first observations of very weak emission from slow-moving ejecta up to 2 cm from the target and times extending to {approx}1.5 ms. Time-of-flight velocities inferred from the emission measurements indicate velocities (v {approximately} (0.45--1.2) {times} 10{sup 4} cm s{sup {minus}1}) comparable to those measured for the large particles which often accompany the pulsed laser deposition process. Gated photon counting is employed to obtain temporally resolved spectra of this weak emission. The spectral shape is characteristic of blackbody emission, which shifts to longer wavelengths as the particles cool during flight in vacuum. Estimates of the temperature of the particles are made based on the emissivity of a perfect blackbody and range from 2200 K to 3200 K for both BN and YBCO when irradiated at ({Phi}{sub 248} = 3.5 J cm{sup {minus}2} and 1.5 J cm{sup {minus}2}, respectively. The temperature decrease of the particles in vacuum is compared to a radiative cooling model which gives estimates of the initial surface temperature and radii of the particles.

A novel field measurement method for determining fine particle and gas emissions from residential wood combustion

Science.gov (United States)

Tissari, Jarkko; Hytönen, Kati; Lyyränen, Jussi; Jokiniemi, Jorma

Emission data from residential wood combustion are usually obtained on test stands in the laboratory but these measurements do not correspond to the operational conditions in the field because of the technological boundary conditions (e.g. testing protocol, environmental and draught conditions). The field measurements take into account the habitual practice of the operators and provide the more reliable results needed for emission inventories. In this study, a workable and compact method for measuring emissions from residential wood combustion in winter conditions was developed. The emissions for fine particle, gaseous and PAH compounds as well as particle composition in real operational conditions were measured from seven different appliances. The measurement technique worked well and was evidently suitable for winter conditions. It was easy and fast to use, and no construction scaffold was needed. The dilution of the sample with the combination of a porous tube diluter and an ejector diluter was well suited to field measurement. The results indicate that the emissions of total volatile organic carbon (TVOC) (17 g kg -1 (of dry wood burned)), carbon monoxide (CO) (120 g kg -1) and fine particle mass (PM 1) (2.7 g kg -1) from the sauna stove were higher than in the other measured appliances. In the masonry heaters, baking oven and stove, the emissions were 2.9-9 g kg -1 TVOC, 28-68 g kg -1 CO and 0.6-1.6 g kg -1 PM 1. The emission of 12 PAHs (PAH 12) from the sauna stove was 164 mg kg -1 and consisted mainly of PAHs with four benzene rings in their structure. PAH 12 emission from other appliances was, on average, 21 mg kg -1 and was dominated by 2-ring PAHs. These results indicate that despite the non-optimal operational practices in the field, the emissions did not differ markedly from the laboratory measurements.

Iron solubility related to particle sulfur content in source emission and ambient fine particles.

Science.gov (United States)

Oakes, M; Ingall, E D; Lai, B; Shafer, M M; Hays, M D; Liu, Z G; Russell, A G; Weber, R J

2012-06-19

The chemical factors influencing iron solubility (soluble iron/total iron) were investigated in source emission (e.g., biomass burning, coal fly ash, mineral dust, and mobile exhaust) and ambient (Atlanta, GA) fine particles (PM2.5). Chemical properties (speciation and mixing state) of iron-containing particles were characterized using X-ray absorption near edge structure (XANES) spectroscopy and micro-X-ray fluorescence measurements. Bulk iron solubility (soluble iron/total iron) of the samples was quantified by leaching experiments. Major differences were observed in iron solubility in source emission samples, ranging from low solubility (iron solubility did not correspond to silicon content or Fe(II) content. However, source emission and ambient samples with high iron solubility corresponded to the sulfur content observed in single particles. A similar correspondence between bulk iron solubility and bulk sulfate content in a series of Atlanta PM2.5 fine particle samples (N = 358) further supported this trend. In addition, results of linear combination fitting experiments show the presence of iron sulfates in several high iron solubility source emission and ambient PM2.5 samples. These results suggest that the sulfate content (related to the presence of iron sulfates and/or acid-processing mechanisms by H(2)SO(4)) of iron-containing particles is an important proxy for iron solubility.

The Particle Number Emission Characteristics of the Diesel Engine with a Catalytic Diesel Particle Filter

Directory of Open Access Journals (Sweden)

Li Jia Qiang

2016-01-01

Full Text Available Due to their adverse health effects and their abundance in urban areas, diesel exhaust ultrafine particles caused by the aftertreatment devices have been of great concern in the past years. An experiment of particles number emissions was carried out on a high-pressure, common rail diesel engine with catalytic diesel particle filter (CDPF to investigate the impact of CDPF on the number emission characteristics of particles. The results indicated that the conversion rates of CDPF is over 97%. The size distributions of particles are bimodal lognormal distributions downstream CDPF at 1400 r/min and 2300 r/min. CDPF has a lower conversion rates on the nucleation mode particles. The geometric number mean diameters of particles downstream CDPF is smaller than that upstream CDPF.

Particle emission in the hydrodynamical description of relativistic nuclear collisions

International Nuclear Information System (INIS)

Grassi, F.; Hama, Y.; Kodama, T.

1994-09-01

Continuous particle emission during the whole expansion of thermalized matter is studied and a new formula for the observed transverse mass spectrum is derived. In some limit, the usual emission at freeze out scenario (Cooper-Frye formula) may be recovered. In a simplified description of expansion, it is shown that continuous particle emission can lead to a sizable curvature in the pion transverse mass spectrum and parallel slopes for the various particles. These results are compared to experimental data. (author). 26 refs, 3 figs

FAST DIFFERENTIAL EMISSION MEASURE INVERSION OF SOLAR CORONAL DATA

Energy Technology Data Exchange (ETDEWEB)

Plowman, Joseph; Kankelborg, Charles; Martens, Petrus [Montana State University, Bozeman, MT 59717 (United States)

2013-07-01

We present a fast method for reconstructing differential emission measures (DEMs) using solar coronal data. The method consists of a fast, simple regularized inversion in conjunction with an iteration scheme for removal of residual negative emission measure. On average, it computes over 1000 DEMs s{sup -1} for a sample active region observed by the Atmospheric Imaging Assembly (AIA) on the Solar Dynamics Observatory, and achieves reduced chi-squared of order unity with no negative emission in all but a few test cases. The high performance of this method is especially relevant in the context of AIA, which images of order one million solar pixels per second. This paper describes the method, analyzes its fidelity, compares its performance and results with other DEM methods, and applies it to an active region and loop observed by AIA and by the Extreme-ultraviolet Imaging Spectrometer on Hinode.

Physical characterization of the fine particle emissions from commercial aircraft engines during the Aircraft Particle Emissions eXperiment (APEX) 1-3

Science.gov (United States)

Kinsey, John S.; Dong, Yuanji; Williams, D. Craig; Logan, Russell

2010-06-01

The fine particulate matter (PM) emissions from nine commercial aircraft engine models were determined by plume sampling during the three field campaigns of the Aircraft Particle Emissions Experiment (APEX). Ground-based measurements were made primarily at 30 m behind the engine for PM mass and number concentration, particle size distribution, and total volatile matter using both time-integrated and continuous sampling techniques. The experimental results showed a PM mass emission index (EI) ranging from 10 to 550 mg kg -1 fuel depending on engine type and test parameters as well as a characteristic U-shaped curve of the mass EI with increasing fuel flow for the turbofan engines tested. Also, the Teflon filter sampling indicated that ˜40-80% of the total PM mass on a test-average basis was comprised of volatile matter (sulfur and organics) for most engines sampled. The number EIs, on the other hand, varied from ˜10 15 to 10 17 particles kg -1 fuel with the turbofan engines exhibiting a logarithmic decay with increasing fuel flow. Finally, the particle size distributions of the emissions exhibited a single primary mode that were lognormally distributed with a minor accumulation mode also observed at higher powers for all engines tested. The geometric (number) mean particle diameter ranged from 9.4 to 37 nm and the geometric standard deviation ranged from 1.3 to 2.3 depending on engine type, fuel flow, and test conditions.

Mechanism of enhancement of controllable secondary-electron emission from fast single electrons

International Nuclear Information System (INIS)

Lorikyan, M.P.; Kavalov, R.L.; Trofimchuk, N.N.; Arvanov, A.N.; Gavalyan, V.G.

For porous KCl films (density approximately 2 percent, thickness 50-400 μm), the controllable secondary electron emission (CSEE) from fast single electrons with energies of 0.7-2 MeV was studied. An electric field E of approximately 10 4 -10 5 V/cm was set up inside the porous films and the emission curves anti sigma = f(E) and the energy spectra of the secondary electrons were measured. The mean emission coefficient anti sigma increases with increasing E, reaching a value of anti sigma approximately equal to 230. Internal enhancement of CSEE under the action of the E field is explained by a process similar to the Townsend semi-self-maintained discharge in gases. The mean free path L/sub e/ of the secondary electrons estimated on the basis of this mechanism of CSEE enhancement is in good agreement with the L/sub e/ value obtained independently from the energy spectra of the secondary electrons. The report examines the effect of the first critical potential U/sub il/ and of the electron affinity of the dielectric α on the formation of CSEE from a porous dielectric film. The possibility of using such films in particle detectors is discussed

Fast Multispectral Radiometry for Particles Analysis

International Nuclear Information System (INIS)

Sharon, A.; Halevy, I.; Sattinger, D.; Yaar, I.; Krantz, L.; Pinhas, M.

2014-01-01

The radiological risk following detonation of radiological dispersal device (RDD) is highly depends the final particles’ size distribution remains after the detonation. In order to produce a realistic source term for the atmospheric dispersion model we should be able to predict the total fraction of aerosols created after the detonation as well as the respirable part of this fraction. The rest of the particles will not be dispersed downwind and hence them concentration will be calculated using much simpler models. The radiological risk out of radioactive (RA) material is highly depends on the particle size. Respirable size (<10 microns) of Alfa, Beta and Gamma emitters are all dangerous when inhaled into the body while larger aerosolos might be risky from a distance (Gamma emitters) or in an external body contact (Alfa, Beta and Gamma). Larger particles (which are not aerosols) are dangerous as fragments when penetrating the body (Alfa, Beta and Gamma) or when depositing on the ground as Gamma emitters. We show here that by using a fast multispectral radiometryfor the detonation fireball analysis it is possible to quantify the reduction of total amount of aerosols due to particles agglomeration with dirt

Fast Radio Bursts’ Emission Mechanism: Implication from Localization

Energy Technology Data Exchange (ETDEWEB)

Lyutikov, Maxim [Department of Physics and Astronomy, Purdue University, 525 Northwestern Avenue, West Lafayette, IN 47907-2036 (United States)

2017-03-20

We argue that the localization of the repeating fast radio bursts (FRBs) at ∼1 Gpc excludes a rotationally powered type of radio emission (e.g., analogs of Crab’s giant pulses coming from very young energetic pulsars) as the origin of FRBs.

Fast Radio Bursts’ Emission Mechanism: Implication from Localization

International Nuclear Information System (INIS)

Lyutikov, Maxim

2017-01-01

We argue that the localization of the repeating fast radio bursts (FRBs) at ∼1 Gpc excludes a rotationally powered type of radio emission (e.g., analogs of Crab’s giant pulses coming from very young energetic pulsars) as the origin of FRBs.

Photon emission produced by particle-surface collisions

International Nuclear Information System (INIS)

White, C.W.; Tolk, N.H.

1976-02-01

Visible, ultraviolet, and infrared optical emission results from low-energy (20 eV-10 keV) particle-surface collisions. Several distinct kinds of collision induced optical radiation are discussed which provide fundamental information on particle-solid collision processes. Line radiation arises from excited states of sputtered surface constituents and backscattered beam particles. This radiation uniquely identifies the quantum state of sputtered or reflected particles, provides a method for identifying neutral atoms sputtered from the surface, and serves as the basis for a sensitive surface analysis technique. Broadband radiation from the bulk of the solid is attributed to the transfer of projectile energy to the electrons in the solid. Continuum emission observed well in front of transition metal targets is believed to arise from excited atom clusters (diatomic, triatomic, etc.) ejected from the solid in the sputtering process. Application of sputtered atom optical radiation for surface and depth profile analysis is demonstrated for the case of submonolayer quantities of chromium on silicon and aluminum implanted in SiO 2

[Particle emission characteristics of diesel bus fueled with bio-diesel].

Science.gov (United States)

Lou, Di-Ming; Chen, Feng; Hu, Zhi-Yuan; Tan, Pi-Qiang; Hu, Wei

2013-10-01

With the use of the Engine Exhaust Particle Sizer (EEPS), a study on the characteristics of particle emissions was carried out on a China-IV diesel bus fueled with blends of 5% , 10% , 20% , 50% bio-diesel transformed from restaurant waste oil and China-IV diesel (marked separately by BD5, BD10, BD20, BD50), pure bio-diesel (BD100) and pure diesel (BD0). The results indicated that particulate number (PN) and mass (PM) emissions of bio-diesel blends increased with the increase in bus speed and acceleration; with increasing bio-diesel content, particulate emissions displayed a relevant declining trend. In different speed ranges, the size distribution of particulate number emissions (PNSD) was bimodal; in different acceleration ranges, PNSD showed a gradual transition from bimodal shape to unimodal when bus operation was switched from decelerating to accelerating status. Bio-diesel blends with higher mixture ratios showed significant reduction in PN emissions for accumulated modes, and the particulate number emission peaks moved towards smaller sizes; but little change was obtained in PN emissions for nuclei modes; reduction also occurred in particle geometric diameter (Dg).

Ion-induced emission of charged particles from solid hydrogen and deuterium

International Nuclear Information System (INIS)

Borgesen, P.; Schou, J.; Sorensen, H.

1980-01-01

Measurements have been made of the emission of both positive and negative particles from solid hydrogen and deuterium for normal incidence of H + , H + 2 , H + 3 , D 2 H + , D + 3 and He + ions up to 10 keV. For positive particles the emission coefficient increased with increasing energy of incidence to reach a value of 0.08 per atom for 10 keV H + onto hydrogen. Apparently the positive particles are sputtered ones. The negative particles emitted are predominantly electrons. The emission coefficient per incident atom as a function of the velocity of the incident particle agress fairly well with results published earlier for incidence of hydrogen and deuterium ions. However, systematic differences of up to 10% are now observed between the coefficients for the different types of ions. (orig.)

Fast hisslers: a form of magnetospheric radio emissions

International Nuclear Information System (INIS)

Siren, J.C.

1974-01-01

Auroral radio hiss bursts in the frequency range 2-18 kHz have been observed, with rise or turn-on-times of 20-50 ms, and fall or turn-off times of 20-80 ms. These time scales are too brief to reconcile with the Cerenkov radiation emission mechanism often proposed as the transducer that converts precipitating auroral electron kinetic energy into very-low-frequency radio wave energy. The auroral hiss bursts, called here ''fast hisslers,'' are observed to be ''dispersed,', that is, their arrival time at the receiving site is not simultaneous at all frequencies, but depends on frequency in a way that is consistent with propagation in the whistler mode of electromagnetic wave propagation. Since whistler mode wave propagation at these frequencies occurs only in the earth' magnetosphere, it is inferred that these fast hisslers are of magnetospheric origin. On the assumption that all the observed dispersion results from whistler mode dispersion at high latitudes, altitudes of origin of 1800 km to 30,000 km are calculated for these emissions. Fine details of some of the amplitude spectra of fast hisslers have been examined. Potential double layers have been investigated as a highly localized region of acceleration of the auroral electrons that are believed to be the source of energy of the fast hisslers. Evidence is strong that a plasma instability exists which rapidly converts electron kinetic energies into whistler-mode wave energy traveling in the same direction relative to the rest frame of the thermal magnetospheric plasma

Light absorption by primary particle emissions from a lignite burning plant

International Nuclear Information System (INIS)

Bond, T.C.; Bussemer, M.; Wehner, B.; Keller, S.; Charlson, R.J.; Heintzenberg, J.

1999-01-01

Anthropogenic aerosols from the burning of fossil fuels contribute to climate forcing by both scattering and absorbing solar radiation, and estimates of climate forcing by light-absorbing primary particles have recently been published. While the mass and optical properties of emissions are needed for these studies, the available measurements do not characterize the low-technology burning that is thought to contribute a large fraction of light-absorbing material to the global budget. The authors have measured characteristics of particulate matter (PM) emitted from a small, low-technology lignite-burning plant. The PM emission factor is comparable to those used to calculate emission inventories of light-absorbing particles. However, the fine fraction, the absorbing fraction, and the absorption efficiency of the emissions are substantially below assumptions that have been made in inventories of black carbon emissions and calculations of climate forcing. The measurements suggest that nonblack, light-absorbing particles are emitted from low-technology coal burning. As the burning rate increases, the emitted absorption cross-section decreases, and the wavelength dependence of absorption becomes closer to that of black particles

Measurements and computer modeling of fast ion emission from plasma accelerators of the rod plasma injector type

International Nuclear Information System (INIS)

Malinowski, Karol; Sadowski, Marek J; Skladnik-Sadowska, Elzbieta

2014-01-01

This paper reports on the results of experimental studies and computer simulations of the emission of fast ion streams from so-called rod plasma injectors (RPI). Various RPI facilities have been used at the National Centre for Nuclear Research (NCBJ) for basic plasma studies as well as for material engineering. In fact, the RPI facilities have been studied experimentally for many years, particularly at the Institute for Nuclear Sciences (now the NCBJ), and numerous experimental data have been collected. Unfortunately, the ion emission characteristics have so far not been explained theoretically in a satisfactory way. In this paper, in order to explain these characteristics, use was made of a single-particle model. Taking into account the stochastic character of the ion emission, we applied a Monte Carlo method. The performed computer simulations of a pinhole image and energy spectrum of deuterons emitted from RPI-IBIS, which were computed on the basis of the applied model, appeared to be in reasonable agreement with the experimental data. (paper)

Size-resolved particle emission factors for individual ships

Science.gov (United States)

Jonsson, Åsa M.; Westerlund, Jonathan; Hallquist, Mattias

2011-07-01

In these experiments size-resolved emission factors for particle number (EFPN) and mass (EFPM) have been determined for 734 individual ship passages for real-world dilution. The method used is an extractive sampling method of the passing ship plumes where particle number/mass and CO2 were measured with high time resolution (1 Hz). The measurements were conducted on a small island located in the entrance to the port of Gothenburg (N57.6849, E11.838), the largest harbor in Scandinavia. This is an emission control area (ECA) and in close vicinity to populated areas. The average EFPN and EFPM were 2.55 ± 0.11 × 1016 (kg fuel)-1 and 2050 ± 110 mg (kg fuel)-1, respectively. The determined EF for ships with multiple passages showed a great reproducibility. Size-resolved EFPN were peaking at small particle sizes ˜35 nm. Smaller particle sizes and hence less mass were observed by a gas turbine equipped ship compared to diesel engine equipped ships. On average 36 to 46% of the emitted particles by number were non-volatile and 24% by mass (EFPN 1.16 ± 0.19 × 1016 [kg fuel]-1 and EFPM 488 ± 73 mg [kg fuel]-1, respectively). This study shows a great potential to gain large data-sets regarding ship emission determining parameters that can improve current dispersion modeling for health assessments on local and regional scales. The global contributions of total and non-volatile particle mass from shipping using this extensive data-set from an ECA were estimated to be at least 0.80 Tgy-1 and 0.19 Tgy-1.

Characteristics of the fast electron emission produced during the ...

Indian Academy of Sciences (India)

water adsorption and other characteristics of the fast electron emission ..... that the surface charges which leak away when there is adosrbed water on ... implies that it is a measure of the supply of excited species rather than due to the charge.

Signature of intermittent behavior in the emission spectra of target associated particles from 84Kr-AgBr interactions at 0.95 GeV/A

International Nuclear Information System (INIS)

Bhattacharjee, B.; Sengupta, S.; Mukhopadhyay, A.; Singh, V.

2004-01-01

In this report an attempt has been made to study, by studying the fluctuation in spatial distribution in χ(cosθ) space, the intermittent behaviour and fractal properties of emission spectra of fast and slow target associated particles from 84 Kr-AgBr interactions at 0.95 GeV/A

Particle Emissions from Biomass Combustion

Energy Technology Data Exchange (ETDEWEB)

Szpila, Aneta; Bohgard, Mats [Lund Inst. of Technology (Sweden). Div. of Ergonomics and Aerosol Technology; Strand, Michael; Lillieblad, Lena; Sanati, Mehri [Vaexjoe Univ. (Sweden). Div. of Bioenergy Technology; Pagels, Joakim; Rissler, Jenny; Swietlicki, Erik; Gharibi, Arash [Lund Univ. (Sweden). Div. of Nuclear Physics

2003-05-01

particle number concentration increased slightly with increasing load, at the same time the fine mode particles became smaller. This was probably caused by different degree of particle coagulation as the residence time in the boiler was changed. The mean diameter during combustion of forest residue was around 100 nm compared to 70-80 nm for dry wood and pellets, while the total number was close to constant. This explains the differences in mass concentration found in the impactor measurements. The concentrations of CO and THC was highest for the dry wood fuel, the PAH concentration was highest for pellets combustion in boiler 4, however this boiler was poorly tuned at the time of measurement. The PAH concentration was 5 times higher during combustion of dry wood compared to forest residue. The concentration of CO, THC and PAH varied to a great extend. The high concentrations were measured in boilers running at a low load. The concentration of particle organic carbon was less than 15% of PMI for all fuels. However we used heated primary dilution, which inhibits the condensation of organic components into, the particle phase. A significant fraction of the emitted organic carbon may condense to the particle phase during dilution after the stack or after being oxidized in the atmosphere. We also measured elemental carbon in the particle phase. The contribution to PM1 was as high as 25-30% during pellets combustion at low load and 8% at low load during combustion of dry wood. In all other cases the EC-concentration was less than 3% of PMI. PIXE and lon-chromatography confirmed that alkali-salts were the dominant chemical species. PIXE analysis revealed that emitted amounts of heavy metals such as Zn, Cd and Pb are strongly dependent on the type of the fuel used. Forest residues gave high emissions of Zn, Cd and Pb, while pellets gave very high emissions of Cd and Zn. The fuel with the lowest emissions of heavy metals was dry wood. This again could be related to ash content in

Hazard assessment of exhaust emissions - The next generation of fast and reliable tools for in vitro screening

Science.gov (United States)

Rothen-Rutishauser, B.

2017-12-01

Hazard assessment of exhaust emissions - The next generation of fast and reliable tools for in vitro screening Barbara Rothen-Rutishauser Adolphe Merkle Institute, University of Fribourg, Switzerland; barbara.rothen@unifr.ch Pollution by vehicles is a major problem for the environment due to the various components in the exhaust gasses that are emitted into the atmosphere. A large number of epidemiological studies demonstrate the profound impact of vehicle emissions upon human health [1-3]. Such studies however, are unable to attribute a given subset of emissions to a certain adverse effect, which renders decision making difficult. Standardized protocols for exhaust toxicity assessment are lacking and it relies in many aspects on epidemiological and in vivo studies (animals), which are very time and cost-intensive and suffer from considerable ethical issues. An overview about the current state of research and clinical aspects in the field, as well as about the development of sophisticated in vitro approaches mimicking the inhalation of airborne particles / exhaust for the toxicological testing of engine emissions will be provided. Data will be presented that show that the combination of an air-liquid exposure system and 3D lung-cell culture model offers an adequate tool for fast and reliable investigations of complete exhaust toxicity as well as the effects of particulate fraction [4,5]. This approach yields important results for novel and improved emission technologies in the early stages of product development. [1] Donaldson et al. Part Fibre Toxicol 2005, 2: 10. [2] Ghio et al. J Toxicol Environ Health B Crit Rev 2012, 15: 1-21. [3] Peters et al. Res Rep Health Eff Inst 2009, 5-77. [4] Bisig et al. Emiss Control Sci Technol 2015, 1: 237-246. [5] Steiner et al. Atmos Environ 2013, 81: 380-388.

Influence of field emission on the propagation of cylindrical fast ionization wave in atmospheric-pressure nitrogen

Energy Technology Data Exchange (ETDEWEB)

Levko, Dmitry; Raja, Laxminarayan L. [Department of Aerospace Engineering and Engineering Mechanics, The University of Texas at Austin, Austin, Texas 78712 (United States)

2016-04-21

The influence of field emission of electrons from surfaces on the fast ionization wave (FIW) propagation in high-voltage nanosecond pulse discharge in the atmospheric-pressure nitrogen is studied by a one-dimensional Particle-in-Cell Monte Carlo Collisions model. A strong influence of field emission on the FIW dynamics and plasma parameters is obtained. Namely, the accounting for the field emission makes possible the bridging of the cathode–anode gap by rather dense plasma (∼10{sup 13 }cm{sup −3}) in less than 1 ns. This is explained by the generation of runaway electrons from the field emitted electrons. These electrons are able to cross the entire gap pre-ionizing it and promoting the ionization wave propagation. We have found that the propagation of runaway electrons through the gap cannot be accompanied by the streamer propagation, because the runaway electrons align the plasma density gradients. In addition, we have obtained that the field enhancement factor allows controlling the speed of ionization wave propagation.

[Ultrafine particle number concentration and size distribution of vehicle exhaust ultrafine particles].

Science.gov (United States)

Lu, Ye-qiang; Chen, Qiu-fang; Sun, Zai; Cai, Zhi-liang; Yang, Wen-jun

2014-09-01

Ultrafine particle (UFP) number concentrations obtained from three different vehicles were measured using fast mobility particle sizer (FMPS) and automobile exhaust gas analyzer. UFP number concentration and size distribution were studied at different idle driving speeds. The results showed that at a low idle speed of 800 rmin-1 , the emission particle number concentration was the lowest and showed a increasing trend with the increase of idle speed. The majority of exhaust particles were in Nuclear mode and Aitken mode. The peak sizes were dominated by 10 nm and 50 nm. Particle number concentration showed a significantly sharp increase during the vehicle acceleration process, and was then kept stable when the speed was stable. In the range of 0. 4 m axial distance from the end of the exhaust pipe, the particle number concentration decayed rapidly after dilution, but it was not obvious in the range of 0. 4-1 m. The number concentration was larger than the background concentration. Concentration of exhaust emissions such as CO, HC and NO showed a reducing trend with the increase of idle speed,which was in contrast to the emission trend of particle number concentration.

Positron Emission Tomography Particle tracking using cluster analysis

International Nuclear Information System (INIS)

Gundogdu, O.

2004-01-01

Positron Emission Particle Tracking was successfully used in a wide range of industrial applications. This technique primarily uses a single positron emitting tracer particle. However, using multiple particles would provide more comparative information about the physical processes taking place in a system such as mixing or fluidised beds. In this paper, a unique method that enables us to track more than one particle is presented. This method is based on the midpoint of the closest distance between two trajectories or coincidence vectors. The technique presented in this paper employs a clustering method

Positron Emission Tomography Particle tracking using cluster analysis

Energy Technology Data Exchange (ETDEWEB)

Gundogdu, O. [University of Birmingham, School of Physics and Astronomy, Birmingham, B15 2TT (United Kingdom)]. E-mail: o.gundogdu@surrey.ac.uk

2004-12-01

Positron Emission Particle Tracking was successfully used in a wide range of industrial applications. This technique primarily uses a single positron emitting tracer particle. However, using multiple particles would provide more comparative information about the physical processes taking place in a system such as mixing or fluidised beds. In this paper, a unique method that enables us to track more than one particle is presented. This method is based on the midpoint of the closest distance between two trajectories or coincidence vectors. The technique presented in this paper employs a clustering method.

[Air Dielectric Barrier Discharge Emission Spectrum Measurement and Particle Analysis of Discharge Process].

Science.gov (United States)

Shen, Shuang-yan; Jin, Xing; Zhang, Peng

2016-02-01

The emission spectrum detection and diagnosis is one of the most common methods of application to the plasma. It provides wealth of information of the chemical and physical process of the plasma. The analysis of discharge plasma dynamic behavior plays an important role in the study of gas discharge mechanism and application. An air dielectric discharge spectrum measuring device was designed and the emission spectrum data was measured under the experimental condition. The plasma particles evolution was analyzed from the emission spectrum. The numerical calculation model was established and the density equation, energy transfer equation and the Boltzmann equation was coupled to analyze the change of the particle density to explain the emission spectrum characteristics. The results are that the particle density is growing with the increasing of reduced electric field. The particle density is one or two orders of magnitude difference for the same particle at the same moment for the reduced electric field of 40, 60 or 80 Td. A lot of N₂ (A³), N₂ (A³) and N₂ (C³) particles are generated by the electric field excitation. However, it transforms quickly due to the higher energy level. The transformation returns to the balance after the discharge of 10⁻⁶ s. The emission spectrometer measured in the experiments is mostly generated by the transition of excited nitrogen. The peak concentration of O₂ (A¹), O₂ (B¹) and O₂ (A³ ∑⁺u) is not low compared to the excited nitrogen molecules. These particles energy is relatively low and the transition spectral is longer. The spectrometer does not capture the oxygen emission spectrum. And the peak concentration of O particles is small, so the transition emission spectrum is weak. The calculation results of the stabled model can well explain the emission spectrum data.

Size-resolved particle number emission patterns under real-world driving conditions using positive matrix factorization.

Science.gov (United States)

Domínguez-Sáez, Aida; Viana, Mar; Barrios, Carmen C; Rubio, Jose R; Amato, Fulvio; Pujadas, Manuel; Querol, Xavier

2012-10-16

A novel on-board system was tested to characterize size-resolved particle number emission patterns under real-world driving conditions, running in a EURO4 diesel vehicle and in a typical urban circuit in Madrid (Spain). Emission profiles were determined as a function of driving conditions. Source apportionment by Positive Matrix Factorization (PMF) was carried out to interpret the real-world driving conditions. Three emission patterns were identified: (F1) cruise conditions, with medium-high speeds, contributing in this circuit with 60% of total particle number and a particle size distribution dominated by particles >52 nm and around 60 nm; (F2) transient conditions, stop-and-go conditions at medium-high speed, contributing with 25% of the particle number and mainly emitting particles in the nucleation mode; and (F3) creep-idle conditions, representing traffic congestion and frequent idling periods, contributing with 14% to the total particle number and with particles in the nucleation mode (emissions depending on particle size and driving conditions. Differences between real-world emission patterns and regulatory cycles (NEDC) are also presented, which evidence that detecting particle number emissions real-world driving conditions.

Delta-electron emission in fast heavy ion atom collisions

International Nuclear Information System (INIS)

Schmidt-Boecking, H.; Ramm, U.; Berg, H.; Kelbch, C.; Feng Jiazhen; Hagmann, S.; Kraft, G.; Ullrich, J.

1991-01-01

The δ-electron emission processes occuring in fast heavy ion atom collisons are explained qualitatively. The different spectral structures of electron emission arising from either the target or the projectile are explained in terms of simple models of the kinetics of momentum transfer induced by the COULOMB forces. In collisions of very heavy ions with matter, high nuclear COULOMB forces are created. These forces lead to a strong polarization of the electronic states of the participated electrons. The effects of this polarization are discussed. (orig.)

Collisional activation by the fast particle

International Nuclear Information System (INIS)

Hiraoka, Kenzo

1996-01-01

Collisional activation of the matter induced by the bombardment of the fast particle is summarized. The particle with the velocity higher than the Bohr velocity (transit time through 5A shorter than 2.5x10 -16 s) experiences the electronic stopping power when it passes through the matter and induces dense electronic excitations and ionizations which results in the heavy sputtering of the matter. This kind of activation is usefully applied in the PDMS. When the particle velocity becomes lower than the Bohr velocity, the energy is mainly deposited to the matter by the nuclear stopping power, i.e., energy loss is governed by the screened Coulombic collisions of the atoms giving rise to the momentum transfer to the target nuclei. When the transit time of the particle through 5A is between 2.5x10 -16 -10 -14 s, the electronic excitation and ionization take place by the collision. These phenomena are fully utilized in the FAB/SIMS and CID techniques. With the transit time in the range of 10 -14 -2.5x10 -13 s, the velocity is not high enough for the electronic excitation and the particle loses its energy mainly by the vibrational and phonon excitation of the target. This range of the velocity corresponds to that of the massive cluster impact ionization. With the velocity equal to or lower than 2.5x10 -13 s, the energy of the incident particle is consumed mainly by the phonon excitation and the collision results in the modest heating of the colliding interface between the projectile and the target. This range of the velocity is successfully used in the ionized cluster beam technique developed by Takagi of the Kyoto University. (author). 59 refs

Fast particle effects on the internal kink, fishbone and Alfven modes

International Nuclear Information System (INIS)

Gorelenkov, N.N.; Bernabei, S.; Cheng, C.Z.; Fu, G.Y.; Hill, K.; Kaye, S.; Kramer, G.J.; Nazikian, R.; Park, W.; Kusama, Y.; Shinokhara, K.; Ozeki, T.

2001-01-01

The issues of linear stability of low frequency perturbative and nonperturbative modes in advanced tokamak regimes are addressed based on recent developments in theory, computational methods, and progress in experiments. Perturbative codes NOVA and ORBIT are used to calculate the effects of TAEs on fast particle population in spherical tokamak NSTX. Nonperturbative analysis of chirping frequency modes in experiments on TFTR and JT-60U is presented using the kinetic code HINST, which identified such modes as a separate branch of Alfven modes - resonance TAE (R-TAE). Internal kink mode stability in the presence of fast particles is studied using the NOVA code and hybrid kinetic-MHD nonlinear code M3D. (author)

Fast Particle Effects on the Internal Kink, Fishbone and Alfven Modes

International Nuclear Information System (INIS)

Gorelenkov, N.N.; Bernabei, S.; Cheng, C.Z.; Fu, G.Y.; Hill, K.; Kaye, S.; Kramer, G.J.; Kusama, Y.; Shinohara, K.; Nazikian, R.; Ozeki, T.; Park, W.

2000-01-01

The issues of linear stability of low frequency perturbative and nonperturbative modes in advanced tokamak regimes are addressed based on recent developments in theory, computational methods, and progress in experiments. Perturbative codes NOVA and ORBIT are used to calculate the effects of TAEs on fast particle population in spherical tokamak NSTX. Nonperturbative analysis of chirping frequency modes in experiments on TFTR and JT-60U is presented using the kinetic code HINST, which identified such modes as a separate branch of Alfven modes - resonance TAE (R-TAE). Internal kink mode stability in the presence of fast particles is studied using the NOVA code and hybrid kinetic-MHD nonlinear code M3D

Improved field emission performance of carbon nanotube by introducing copper metallic particles

Directory of Open Access Journals (Sweden)

Chen Yiren

2011-01-01

Full Text Available Abstract To improve the field emission performance of carbon nanotubes (CNTs, a simple and low-cost method was adopted in this article. We introduced copper particles for decorating the CNTs so as to form copper particle-CNT composites. The composites were fabricated by electrophoretic deposition technique which produced copper metallic particles localized on the outer wall of CNTs and deposited them onto indium tin oxide (ITO electrode. The results showed that the conductivity increased from 10-5 to 4 × 10-5 S while the turn-on field was reduced from 3.4 to 2.2 V/μm. Moreover, the field emission current tended to be undiminished after continuous emission for 24 h. The reasons were summarized that introducing copper metallic particles to decorate CNTs could increase the surface roughness of the CNTs which was beneficial to field emission, restrain field emission current from saturating when the applied electric field was above the critical field. In addition, it could also improve the electrical contact by increasing the contact area between CNT and ITO electrode that was beneficial to the electron transport and avoided instable electron emission caused by thermal injury of CNTs.

3D fast reconstruction in positron emission tomography

International Nuclear Information System (INIS)

Egger, M.L.; Scheurer, A. Hermann; Joseph, C.; Morel, C.

1996-01-01

The issue of long reconstruction times in positron emission tomography (PET) has been addressed from several points of view, resulting in an affordable dedicated system capable of handling routine 3D reconstructions in a few minutes per frame : on the hardware side using fast processors and a parallel architecture, and on the software side, using efficient implementation of computationally less intensive algorithms

Particle Morphology From Wood-Burning Cook Stoves Emissions

Science.gov (United States)

Peralta, O.; Carabali, G.; Castro, T.; Torres, R.; Ruiz, L. G.; Molina, L. T.; Saavedra, I.

2013-12-01

Emissions from three wood-burning cook stoves were sampled to collect particles. Transmission electron microscope (TEM) copper grids were placed on the last two stages of an 8-stage MOUDI cascade impactor (d50= 0.32, and 0.18 μm). Samples were obtained on two heating stages of cooking, the first is a quick heating process to boil 1 liter of water, and the second is to keep the water at 90 C. Absorption coefficient, scattering coefficients, and particles concentration (0.01 - 2.5 μm aerodynamic diameter) were measured simultaneously using an absorption photometer (operated at 550 nm), a portable integrating nephelometer (at 530 nm), and a condensation particle counter connected to a chamber to dilute the wood stoves emissions. Transmission electron micrographic images of soot particles were acquired at different magnifications using a High Resolution Transmission Electron Microscope (HRTEM) JEOL HRTEM 4000EX operating at 200 kV, equipped with a GATAN digital micrograph system for image acquisition. The morphology of soot particles was analyzed calculating the border-based fractal dimension (Df). Particles sampled on the first heating stage exhibit complex shapes with high values of Df, which are present as aggregates formed by carbon ceno-spheres. The presence of high numbers of carbon ceno-spheres can be attributed to pyrolysis, thermal degradation, and others processes prior to combustion. Energy dispersive X-ray spectroscopy (EDS) was used to determine the elemental composition of particles. EDS analysis in particles with d50= 0.18 μm showed a higher content of carbonaceous material and relevant amounts of Si, S and K.

Fast Plasma Potential Measurements Using an Emissive Probe

Science.gov (United States)

Ready, Amanda; Clark, Michael; Endrizzi, Douglass; Forest, Cary; Peterson, Ethan

2017-10-01

A heated emissive probe was developed for making direct plasma potential (Vp) measurements in rapidly fluctuating plasmas. Previous experiments on the Big Red Ball (BRB) were hindered by sudden potential drops, making Langmuir measurements of the plasma potential difficult. DC heating of a tungsten filament to emission allowed for fast (4 MHz) floating potential measurements that closely matched Vp. Two BRB experiments currently use the emissive probe. The investigation of unmagnetized, collisionless shocks used plasma potential measurements to study the sub-structure of strong plasma shocks. A separate investigation of emulated magnetospheres in laboratory plasmas used the plasma potential to map the equilibria and instabilities in the electric field of such structures. Results showing electric field measurements and comparison with cold Langmuir measurements will be presented. Future plans for probe modifications and applications to other experiments on the BRB will also be shown.

Spot: a new Monte Carlo solver for fast alpha particles

International Nuclear Information System (INIS)

Schneider, M.; Eriksson, L.G.; Basiuk, V.; Imbeaux, F.

2004-01-01

The predictive transport code CRONOS has been augmented by an orbit following Monte Carlo code, SPOT (Simulation of Particle Orbits in a Tokamak). The SPOT code simulates the dynamics of nonthermal particles, and takes into account effects of finite orbit width and collisional transport of fast ions. Recent developments indicate that it might be difficult to avoid, at least transiently, current holes in a reactor. They occur already on existing tokamaks during advanced tokamak scenarios. The SPOT code has been used to study the alpha particle behaviour in the presence of current holes for both JET and ITER relevant parameters. (authors)

Coherent radiation of photon by fast particles in exited matter

International Nuclear Information System (INIS)

Ryazanov, M.I.

1981-01-01

The review on the theory of coherent photon radiation by fast charged particle interaction with excited by external electromagnetic field atoms of matter is presented. The motive particle excites in the matter longitudinal electric oscillations (plasmons, longitudinal optical phonons, longitudinal excitons). Energy and momentum conservation laws in the course of quantum radiation in the matter by a charged particle are considered taking into account the energy-matter exchange. It follows from the conservation laws that for the processes investigated the quantum angle of escape is stiffly connected with its frequency. The cohe-- rent luminescence processes are considered as generalized Vavilov- Cherenkov radiation [ru

'Beam-emission spectroscopy' diagnostics also measure edge fast-ion light

International Nuclear Information System (INIS)

Heidbrink, W W; Bortolon, A; McKee, G R; Smith, D R

2011-01-01

Beam-emission spectroscopy (BES) diagnostics normally detect fluctuations in the light emitted by an injected neutral beam. Under some circumstances, however, light from fast ions that charge exchange in the high neutral-density region at the edge of the plasma make appreciable contributions to the BES signals. This 'passive' fast-ion D α (FIDA) light appears in BES signals from both the DIII-D tokamak and the National Spherical Torus Experiment (NSTX). One type of passive FIDA light is associated with classical orbits that traverse the edge. Another type is caused by instabilities that expel fast ions from the core; this light can complicate measurement of the instability eigenfunction.

Particle Induced X-ray Emission (PIXE) Approach for the Quantification of Thin Al Films

International Nuclear Information System (INIS)

Younes, G; Zahraman, K; Nsouli, B; Soueidan, M; Ferro, G

2008-01-01

Particle Induced X-ray Emission (PIXE) has been used as a fast and non-destructive technique for sensitive characterization of ultra thin Al films deposited by evaporation onto Si substrate. In this work the PIXE technique was optimized, using proton beam at different energies and different angles of incidence, for the characterization of ultra thin Al films (few nanometers) deposited onto Si substrate. The PIXE results showed that a proton beam of 300 keV under tilting angle of 80 degree permits an accurate determination of Al with high sensitivity within few minutes of acquisition time and a LOD of less than 0.2 nm. The LOD versus energy and tilting angle will be presented and discussed. (author)

Particle induced X-ray emission

International Nuclear Information System (INIS)

Cohen, D.D.

1991-08-01

The accelerator based ion beam technique of Particle Induced X-ray Emission (PIXE) is discussed in some detail. This report pulls together all major reviews and references over the last ten years and reports on PIXE in vacuum and using external beams. The advantages, limitations, costs and types of studies that may be undertaken using an accelerator based ion beam technique such as PIXE, are also discussed. 25 refs., 7 tabs., 40 figs

Effect of electron degeneracy on fast-particles energy deposition in dense plasma systems

International Nuclear Information System (INIS)

Johzaki, T.; Nakao, Y.; Nakashima, H.; Kudo, K.

1997-01-01

The effects of electron degeneracy on fast-particles energy deposition in dense plasmas are investigated by making transport calculations for the fast particles. It is found that the degeneracy substantially affects the profiles of energy deposition of 3.52-MeV α-particles. On the other hand, the effect on the energy deposition of 14.1-MeV neutrons is negligibly small because the recoil ions, which transfer the neutron energy to the plasma constituents, are produced in a whole plasma volume due to the long mean-free-path of neutrons. The coupled transport-hydrodynamic calculations show that these effects of degeneracy are negligible in the ignition and burn characteristics of central ignition D-T targets. (author)

Beta delayed particle emission in light nuclei

International Nuclear Information System (INIS)

Riisager, K.; Gabelmann, H.

1991-01-01

A short discussion of theoretical treatments of beta delayed particle emission is followed by a presentation of data on the newly found beta delayed deuteron decay of 6 He. This decay cannot be described properly with existing theories. (author) 8 refs.; 3 figs

The influence of design and fuel parameters on the particle emissions from wood pellets combustion. Final report

Energy Technology Data Exchange (ETDEWEB)

Wiinikka, Henrik; Gebart, Rikard [Energy Technology Centre, Piteaa (Sweden)

2005-02-01

Combustion of solid biomass under fixed bed conditions is a common technique to generate heat and power in both small and large scale grate furnaces (domestic boilers, stoves, district heating plants). Unfortunately, combustion of biomass will generate particle emissions containing both large fly ash particles and fine particles that consist of fly ash and soot. The large fly ash particles have been produced from fusion of non-volatile ash-forming species in burning char particle. The inorganic fine particles have been produced from nucleation of volatilised ash elements (K, Na, S, Cl and Zn). If the combustion is incomplete, soot particles are also produced from secondary reaction of tar. The particles in the fine fraction grows by coagulation and coalescence to a particle diameter around 0.1 pm. Since the smallest particles are very hard to collect in ordinary cleaning devices they contribute to the ambient air pollution. Furthermore, fine airborne particles have been correlated to adverse effects on the human health. It is therefore essential to minimize particle formation from the combustion process and thereby reduce the emissions of particulates to the ambient air. The aim with this project is to study particle emissions from small scale combustion of wood pellets and to investigate the impact of different operating, construction and fuel parameters on the amount and characteristic of the combustion generated particles. To address these issues, experiments were carried out in a 10 kW updraft fired wood pellets reactor that has been custom designed for systematic investigations of particle emissions. In the flue gas stack, particle emissions were sampled on a filter. The particle mass and number size distributions were analysed by a low pressure cascade impactor and a SMPS (Scanning Electron Mobility Particle Sizer). The results showed that the temperature and the flow pattern in the combustion zone affect the particle emissions. Increasing combustion

Nonlinear interaction of fast particles with Alfven waves in toroidal plasmas

International Nuclear Information System (INIS)

Candy, J.; Borba, D.; Huysmans, G.T.A.; Kerner, W.; Berk, H.L.

1996-01-01

A numerical algorithm to study the nonlinear, resonant interaction of fast particles with Alfven waves in tokamak geometry has been developed. The scope of the formalism is wide enough to describe the nonlinear evolution of fishbone modes, toroidicity-induced Alfven eigenmodes and ellipticity-induced Alfven eigenmodes, driven by both passing and trapped fast ions. When the instability is sufficiently weak, it is known that the wave-particle trapping nonlinearity will lead to mode saturation before wave-wave nonlinearities are appreciable. The spectrum of linear modes can thus be calculated using a magnetohydrodynamic normal-mode code, then nonlinearly evolved in time in an efficient way according to a two-time-scale Lagrangian dynamical wave model. The fast particle kinetic equation, including the effect of orbit nonlinearity arising from the mode perturbation, is simultaneously solved of the deviation, δf = f - f 0 , from an initial analytic distribution f 0 . High statistical resolution allows linear growth rates, frequency shifts, resonance broadening effects, and nonlinear saturation to be calculated quickly and precisely. The results have been applied to an ITER instability scenario. Results show that weakly-damped core-localized modes alone cause negligible alpha transport in ITER-like plasmas--even with growth rates one order of magnitude higher than expected values. However, the possibility of significant transport in reactor-type plasmas due to weakly unstable global modes remains an open question

Geometry and dynamics of particle emission from strongly deformed nuclei

International Nuclear Information System (INIS)

Aleshin, V.P.

1995-01-01

By using our semiclassical approach to particle evaporation from deformed nuclei, we analyze the heuristic models of particle emission from deformed nuclei which are used in the codes GANES, ALICE, and EVAP. The calculations revealed that the heuristic models are reasonable for particle energy spectra but fail, at large deformations, to describe the angular distributions

Monte Carlo simulations of the particle transport in semiconductor detectors of fast neutrons

International Nuclear Information System (INIS)

Sedlačková, Katarína; Zaťko, Bohumír; Šagátová, Andrea; Nečas, Vladimír

2013-01-01

Several Monte Carlo all-particle transport codes are under active development around the world. In this paper we focused on the capabilities of the MCNPX code (Monte Carlo N-Particle eXtended) to follow the particle transport in semiconductor detector of fast neutrons. Semiconductor detector based on semi-insulating GaAs was the object of our investigation. As converter material capable to produce charged particles from the (n, p) interaction, a high-density polyethylene (HDPE) was employed. As the source of fast neutrons, the 239 Pu–Be neutron source was used in the model. The simulations were performed using the MCNPX code which makes possible to track not only neutrons but also recoiled protons at all interesting energies. Hence, the MCNPX code enables seamless particle transport and no other computer program is needed to process the particle transport. The determination of the optimal thickness of the conversion layer and the minimum thickness of the active region of semiconductor detector as well as the energy spectra simulation were the principal goals of the computer modeling. Theoretical detector responses showed that the best detection efficiency can be achieved for 500 μm thick HDPE converter layer. The minimum detector active region thickness has been estimated to be about 400 μm. -- Highlights: ► Application of the MCNPX code for fast neutron detector design is demonstrated. ► Simulations of the particle transport through conversion film of HDPE are presented. ► Simulations of the particle transport through detector active region are presented. ► The optimal thickness of the HDPE conversion film has been calculated. ► Detection efficiency of 0.135% was reached for 500 μm thick HDPE conversion film

Particle emission rates during electrostatic spray deposition of TiO2 nanoparticle-based photoactive coating.

Science.gov (United States)

Koivisto, Antti J; Jensen, Alexander C Ø; Kling, Kirsten I; Kling, Jens; Budtz, Hans Christian; Koponen, Ismo K; Tuinman, Ilse; Hussein, Tareq; Jensen, Keld A; Nørgaard, Asger; Levin, Marcus

2018-01-05

Here, we studied the particle release rate during Electrostatic spray deposition of anatase-(TiO 2 )-based photoactive coating onto tiles and wallpaper using a commercially available electrostatic spray device. Spraying was performed in a 20.3m 3 test chamber while measuring concentrations of 5.6nm to 31μm-size particles and volatile organic compounds (VOC), as well as particle deposition onto room surfaces and on the spray gun user hand. The particle emission and deposition rates were quantified using aerosol mass balance modelling. The geometric mean particle number emission rate was 1.9×10 10 s -1 and the mean mass emission rate was 381μgs -1 . The respirable mass emission-rate was 65% lower than observed for the entire measured size-range. The mass emission rates were linearly scalable (±ca. 20%) to the process duration. The particle deposition rates were up to 15h -1 for deposited particles consisted of mainly TiO 2 , TiO 2 mixed with Cl and/or Ag, TiO 2 particles coated with carbon, and Ag particles with size ranging from 60nm to ca. 5μm. As expected, no significant VOC emissions were observed as a result of spraying. Finally, we provide recommendations for exposure model parameterization. Copyright © 2017 The Author(s). Published by Elsevier B.V. All rights reserved.

Various light particles emissions accompaning light heavy ion collisions

International Nuclear Information System (INIS)

Billerey, R.

1981-01-01

In this work we have investigated light particles emission accompanying heavy-ion induced reactions. The experiments were performed at the isochronous cyclotron of the I.S.N. de Grenoble and we got in and out of plane correlations between solid state and gazeous detectors. In 14 N (100 MeV) + 27 Al we have chosen, light particles emitted in coincidence with deep inelastic fragments or evaporation residues have been measured. Likewise we observed the correlations between fragments and fragments. The particularities we found between protons and alpha emissions are to be assigned to differences in separation energies, but their relative energies and angular momenta have also a significant part [fr

Exhaust particle and NOx emission performance of an SCR heavy duty truck operating in real-world conditions

Science.gov (United States)

Saari, Sampo; Karjalainen, Panu; Ntziachristos, Leonidas; Pirjola, Liisa; Matilainen, Pekka; Keskinen, Jorma; Rönkkö, Topi

2016-02-01

Particle and NOx emissions of an SCR equipped HDD truck were studied in real-world driving conditions using the "Sniffer" mobile laboratory. Real-time CO2 measurement enables emission factor calculation for NOx and particles. In this study, we compared three different emission factor calculation methods and characterised their suitability for real-world chasing experiments. The particle number emission was bimodal and dominated by the nucleation mode particles (diameter below 23 nm) having emission factor up to 1 × 1015 #/kgfuel whereas emission factor for soot (diameter above 23 nm that is consistent with the PMP standard) was typically 1 × 1014 #/kgfuel. The effect of thermodenuder on the exhaust particles indicated that the nucleation particles consisted mainly of volatile compounds, but sometimes there also existed a non-volatile core. The nucleation mode particles are not controlled by current regulations in Europe. However, these particles consistently form under atmospheric dilution in the plume of the truck and constitute a health risk for the human population that is exposed to those. Average NOx emission was 3.55 g/kWh during the test, whereas the Euro IV emission limit over transient testing is 3.5 g NOx/kWh. The on-road emission performance of the vehicle was very close to the expected levels, confirming the successful operation of the SCR system of the tested vehicle. Heavy driving conditions such as uphill driving increased both the NOx and particle number emission factors whereas the emission factor for soot particle number remains rather constant.

Light charged particle emission in heavy-ion reactions – What have ...

Indian Academy of Sciences (India)

coincidence with gamma rays, fission products, evaporation residues have yielded interesting results which bring out the influence of nuclear structure, nuclear mean field and dynamics on the emission of these particles. Keywords. Light charged particles; heavy-ion induced reactions; particle spectra and angular distri-.

Competition between peripheral and central emission in incomplete fusion reactions

International Nuclear Information System (INIS)

Tricoire, H.

1984-01-01

In the frame of a classical model we show that the emission of fast particles in incomplete fusion reactions may occur either from a PEP emission which happens preferentially at low angular momenta or from an inertial emission with a maximum of the cross section located near the critical angular momentum for complete fusion. The competition of these mechanisms depends crucialy of the interaction between the particle to be emitted and the target nucleus. Numerical calculations are performed with various particle target potentials. Using a proximity potential, one gets results in good agreement with experimental data

Energetic-particle-driven instabilities and induced fast-ion transport in a reversed field pinch

International Nuclear Information System (INIS)

Lin, L.; Brower, D. L.; Ding, W. X.; Anderson, J. K.; Capecchi, W.; Eilerman, S.; Forest, C. B.; Koliner, J. J.; Nornberg, M. D.; Reusch, J.; Sarff, J. S.; Liu, D.

2014-01-01

Multiple bursty energetic-particle (EP) driven modes with fishbone-like structure are observed during 1 MW tangential neutral-beam injection in a reversed field pinch (RFP) device. The distinguishing features of the RFP, including large magnetic shear (tending to add stability) and weak toroidal magnetic field (leading to stronger drive), provide a complementary environment to tokamak and stellarator configurations for exploring basic understanding of EP instabilities. Detailed measurements of the EP mode characteristics and temporal-spatial dynamics reveal their influence on fast ion transport. Density fluctuations exhibit a dynamically evolving, inboard-outboard asymmetric spatial structure that peaks in the core where fast ions reside. The measured mode frequencies are close to the computed shear Alfvén frequency, a feature consistent with continuum modes destabilized by strong drive. The frequency pattern of the dominant mode depends on the fast-ion species. Multiple frequencies occur with deuterium fast ions compared to single frequency for hydrogen fast ions. Furthermore, as the safety factor (q) decreases, the toroidal mode number of the dominant EP mode transits from n=5 to n=6 while retaining the same poloidal mode number m=1. The transition occurs when the m=1, n=5 wave-particle resonance condition cannot be satisfied as the fast-ion safety factor (q fi ) decreases. The fast-ion temporal dynamics, measured by a neutral particle analyzer, resemble a classical predator-prey relaxation oscillation. It contains a slow-growth phase arising from the beam fueling followed by a rapid drop when the EP modes peak, indicating that the fluctuation-induced transport maintains a stiff fast-ion density profile. The inferred transport rate is strongly enhanced with the onset of multiple EP modes

Anisotropic and correlated emissions of short range charged particles in anti pAg/Br reactions at 1. 4 GeV/c incident momentum observed in photographic emulsions

Energy Technology Data Exchange (ETDEWEB)

Breivik, F.O.; Jacobsen, T.; Soerensen, S.O.

1984-07-01

Anti pAg/Br reactions at 1.4 GeV/c incident momentum are studied by means of the emulsion technique. A group of short range charged particles is observed. For the events with one short track, a backward and transversal emission is seen, which probably is due to some very fast process. For the events with two short tracks, a back-to-back emission is seen, indicating some two-body decay, where the target nucleus possibly behaves spectator-like.

Anisotropic and correlated emissions of short range charged particles in anti pAg/Br reactions at 1.4 GeV/c incident momentum observed in photographic emulsions

International Nuclear Information System (INIS)

Breivik, F.O.; Jacobsen, T.; Soerensen, S.O.

1984-01-01

Anti pAg/Br reactions at 1.4 GeV/c incident momentum are studied by means of the emulsion technique. A group of short range charged particles is observed. For the events with one short track, a backward and transversal emission is seen, which probably is due to some very fast process. For the events with two short tracks, a back-to-back emission is seen, indicating some two-body decay, where the target nucleus possibly behaves spectator-like. (Auth.)

Fast digital processor for event selection according to particle number difference

International Nuclear Information System (INIS)

Basiladze, S.G.; Gus'kov, B.N.; Li Van Sun; Maksimov, A.N.; Parfenov, A.N.

1978-01-01

A fast digital processor for a magnetic spectrometer is described. It is used in experimental searches for charmed particles. The basic purpose of the processor is discriminating events in the difference of numbers of particles passing through two proportional chambers (PC). The processor consists of three units for detecting signals with PC, and a binary coder. The number of inputs of the processor is 32 for the first PC and 64 for the second. The difference in the number of particles discriminated is from 0 to 8. The resolution time is 180 ns. The processor is built in the CAMAC standard

Acoustic emission during the compaction of brittle UO2 particles

International Nuclear Information System (INIS)

Hegron, Lise

2014-01-01

One of the options considered for recycling minor actinides is to incorporate about 10% to UO 2 matrix. The presence of open pores interconnected within this fuel should allow the evacuation of helium and fission gases to prevent swelling of the pellet and ultimately its interaction with the fuel clad surrounding it. Implementation of minor actinides requires working in shielded cell, reducing their retention and outlawing additions of organic products. The use of fragmentable particles of several hundred micrometers seems a good solution to control the microstructure of the green compacts and thus control the open porosity after sintering. The goal of this study is to monitor the compaction of brittle UO 2 particles by acoustic emission and to link the particle characteristics to the open porosity obtained after the compact sintering. The signals acquired during tensile strength tests on individual granules and compacts show that the acoustic emission allows the detection of the mechanism of fragmentation and enables identification of a characteristic waveform of this fragmentation. The influences of compaction stress, of the initial particle size distribution and of the internal cohesion of the granules, on the mechanical strength of the compact and on the microstructure and open porosity of the sintered pellets, are analyzed. By its ability to identify the range of fragmentation of the granules during compaction, acoustic emission appears as a promising technique for monitoring the compaction of brittle particles in the manufacture of a controlled porosity fuel. (author) [fr

Fast Neutron Emission Tomography of Used Nuclear Fuel Assemblies

Science.gov (United States)

Hausladen, Paul; Iyengar, Anagha; Fabris, Lorenzo; Yang, Jinan; Hu, Jianwei; Blackston, Matthew

2017-09-01

Oak Ridge National Laboratory is developing a new capability to perform passive fast neutron emission tomography of spent nuclear fuel assemblies for the purpose of verifying their integrity for international safeguards applications. Most of the world's plutonium is contained in spent nuclear fuel, so it is desirable to detect the diversion of irradiated fuel rods from an assembly prior to its transfer to ``difficult to access'' storage, such as a dry cask or permanent repository, where re-verification is practically impossible. Nuclear fuel assemblies typically consist of an array of fuel rods that, depending on exposure in the reactor and consequent ingrowth of 244Cm, are spontaneous sources of as many as 109 neutrons s-1. Neutron emission tomography uses collimation to isolate neutron activity along ``lines of response'' through the assembly and, by combining many collimated views through the object, mathematically extracts the neutron emission from each fuel rod. This technique, by combining the use of fast neutrons -which can penetrate the entire fuel assembly -and computed tomography, is capable of detecting vacancies or substitutions of individual fuel rods. This paper will report on the physics design and component testing of the imaging system. This material is based upon work supported by the U.S. Department of Energy, Office of Defense Nuclear Nonproliferation Research and Development within the National Nuclear Security Administration, under Contract Number DE-AC05-00OR22725.

A memory particle model in study of pre-equilibrium emission

International Nuclear Information System (INIS)

Miao rongzhi

1989-01-01

Exciton of a composite system at high energy is divided into two subsystems which consist of memory particle m and non-memory particle r. After introducing α n , the collision factor of m-particle in state n, the coupled master equitions of the occupation probability of state-angle of m-particle and r-particle are established. The expression of state density, taking into account the distinqushability between m-particle and r-particle, and the formulas of the rate of β-particle emission of m-system and r-system in state n are also given. The calculation results show that the fit with experimental data is improved conspicuously and is much better than that obtained from the generalized exciton model

Experimental study of the pion-xenon nucleus collisions without particle production at 3.5 GeV/c momentum: general data

International Nuclear Information System (INIS)

Strugalski, Z.; Pavlak, T.; Pluta, J.

1982-01-01

There exist pion-xenon nucleus collision events in which intensive emission of fast protons, of kinetic energy of about 20-400 MeV, is observed only without particle production. Energy, momentum and angular distributions of the emitted protons are presented and analysed in classes of events with various proton emission intensity. It is concluded that: a)the nucleon emission proceeds independently of the particle production process; b)the observed intensive emission of the ''fast'' protons cannot be treated as a result of a simple knocking-out of the nucleons from the target by the incident hadron

Monte Carlo calculation of secondary electron emission from carbon-surface by obliquely incident particles

International Nuclear Information System (INIS)

Ohya, Kaoru; Kawata, Jun; Mori, Ichiro

1990-01-01

Incidence angle dependences of secondary electron emission from a carbon surface by low energy electron and hydrogen atom are calculated using Monte Carlo simulations on the kinetic emission model. The calculation shows very small increase or rather decrease of the secondary electron yield with oblique incidence. It is explained in terms of not only multiple elastic collisions of incident particles with the carbon atoms but also small penetration depth of the particles comparable with the escape depth of secondary electrons. In addition, the two types of secondary electron emission are distinguished by using the secondary electron yield statistics; one is the emission due to trapped particles in the carbon, and the other is that due to backscattered particles. The high-yield component of the statistics on oblique incidence is more suppressed than those on normal incidence. (author)

Analysis of two colliding laser-produced plasmas by emission spectroscopy and fast photography

Energy Technology Data Exchange (ETDEWEB)

Sanchez-Ake, C., E-mail: citlali.sanchez@ccadet.unam.m [Centro de Ciencias Aplicadas y Desarrollo Tecnologico, Universidad Nacional Autonoma de Mexico, Apartado Postal 70-186, Mexico D.F., C.P. 04510 (Mexico); Mustri-Trejo, D. [Centro de Ciencias Aplicadas y Desarrollo Tecnologico, Universidad Nacional Autonoma de Mexico, Apartado Postal 70-186, Mexico D.F., C.P. 04510 (Mexico); Garcia-Fernandez, T. [Universidad Autonoma de la Ciudad de Mexico, Prolongacion San Isidro 151, Col. San Lorenzo Tezonco, Mexico DF, C.P. 09790 (Mexico); Villagran-Muniz, M. [Centro de Ciencias Aplicadas y Desarrollo Tecnologico, Universidad Nacional Autonoma de Mexico, Apartado Postal 70-186, Mexico D.F., C.P. 04510 (Mexico)

2010-05-15

In this work two colliding laser-induced plasmas (LIP) on Cu and C were studied by means of time resolved emission spectroscopy and fast photography. The experiments were performed using two opposing parallel targets of Cu and C in vacuum, ablated with two synchronized ns lasers. The results showed an increased emission intensity from copper ions Cu II (368.65, 490.97, 493.16, 495.37 and 630.10 nm) and Cu III (374.47 and 379.08 nm) due to the ionization that occurs during collisions of Cu and C species. It was found that the optimum delay between pulses, which yields the maximum emission enhancement of Cu ions, depends on the sampling distance. On the other hand, the emission intensity of C lines, C II (426.70 nm), C III (406.99 and 464.74 nm) and C IV (465.83 nm), decreased and the formation of C{sub 2} molecules was observed. A comparison between the temporal evolution of the individual plasmas and their collision performed by combining imaging and the time resolved emission diagnostics, revealed an increase of the electron temperature and electron density and the splitting of the plume into slow and fast components.

Radiative forcing from particle emissions by future supersonic aircraft

Directory of Open Access Journals (Sweden)

G. Pitari

2008-07-01

Full Text Available In this work we focus on the direct radiative forcing (RF of black carbon (BC and sulphuric acid particles emitted by future supersonic aircraft, as well as on the ozone RF due to changes produced by emissions of both gas species (NO_x, H₂O and aerosol particles capable of affecting stratospheric ozone chemistry. Heterogeneous chemical reactions on the surface of sulphuric acid stratospheric particles (SSA-SAD are the main link between ozone chemistry and supersonic aircraft emissions of sulphur precursors (SO₂ and particles (H₂O–H₂SO₄. Photochemical O₃ changes are compared from four independent 3-D atmosphere-chemistry models (ACMs, using as input the perturbation of SSA-SAD calculated in the University of L'Aquila model, which includes on-line a microphysics code for aerosol formation and growth. The ACMs in this study use aircraft emission scenarios for the year 2050 developed by AIRBUS as a part of the EU project SCENIC, assessing options for fleet size, engine technology (NO_x emission index, Mach number, range and cruising altitude. From our baseline modeling simulation, the impact of supersonic aircraft on sulphuric acid aerosol and BC mass burdens is 53 and 1.5 μg/m², respectively, with a direct RF of −11.4 and 4.6 mW/m² (net RF=−6.8 mW/m². This paper discusses the similarities and differences amongst the participating models in terms of changes to O₃ precursors due to aircraft emissions (NO_x, HO_x,Cl_x,Br_x and the stratospheric ozone sensitivity to them. In the baseline case, the calculated global ozone change is −0.4 ±0.3 DU, with a net radiative forcing (IR+UV of −2.5± 2 mW/m². The fraction of this O₃-RF attributable to SSA-SAD changes is, however, highly variable among the models, depending on the NO_x removal

Profiles of fast ions that are accelerated by high harmonic fast waves in the National Spherical Torus Experiment

International Nuclear Information System (INIS)

Liu, D; Heidbrink, W W; Podesta, M; Ruskov, E; Bell, R E; Fredrickson, E D; Medley, S S; Harvey, R W

2010-01-01

Combined neutral beam injection and high-harmonic fast-wave (HHFW) heating accelerate deuterium fast ions in the National Spherical Torus Experiment (NSTX). With 1.1 MW of HHFW power, the neutron emission rate is about three times larger than in the comparison discharge without HHFW heating. Acceleration of fast ions above the beam injection energy is evident on an E||B type neutral particle analyzer (NPA), a 4-chord solid state neutral particle analyzer (SSNPA) array and a 16-channel fast-ion D-alpha (FIDA) diagnostic. The accelerated fast ions observed by the NPA and SSNPA diagnostics mainly come from passive charge exchange reactions at the edge due to the NPA/SSNPA localization in phase space. The spatial profile of accelerated fast ions that is measured by the FIDA diagnostic is much broader than in conventional tokamaks because of the multiple resonance layers and large orbits in NSTX. The fast-ion distribution function calculated by the CQL3D Fokker-Planck code differs from the measured spatial profile, presumably because the current version of CQL3D uses a zero-banana-width model. In addition, compressional Alfven eigenmode activity is stronger during the HHFW heating and it may affect the fast-ion spatial profile.

A New Paradigm for Flare Particle Acceleration

Science.gov (United States)

Guidoni, Silvina E.; Karpen, Judith T.; DeVore, C. Richard

2017-08-01

The mechanism that accelerates particles to the energies required to produce the observed high-energy impulsive emission and its spectra in solar flares is not well understood. Here, we propose a first-principle-based model of particle acceleration that produces energy spectra that closely resemble those derived from hard X-ray observations. Our mechanism uses contracting magnetic islands formed during fast reconnection in solar flares to accelerate electrons, as first proposed by Drake et al. (2006) for kinetic-scale plasmoids. We apply these ideas to MHD-scale islands formed during fast reconnection in a simulated eruptive flare. A simple analytic model based on the particles’ adiabatic invariants is used to calculate the energy gain of particles orbiting field lines in our ultrahigh-resolution, 2.5D, MHD numerical simulation of a solar eruption (flare + coronal mass ejection). Then, we analytically model electrons visiting multiple contracting islands to account for the observed high-energy flare emission. Our acceleration mechanism inherently produces sporadic emission because island formation is intermittent. Moreover, a large number of particles could be accelerated in each macroscopic island, which may explain the inferred rates of energetic-electron production in flares. We conclude that island contraction in the flare current sheet is a promising candidate for electron acceleration in solar eruptions. This work was supported in part by the NASA LWS and H-SR programs..

Particle and gaseous emissions from individual diesel and CNG buses

Directory of Open Access Journals (Sweden)

Å. M. Hallquist

2013-05-01

Full Text Available In this study size-resolved particle and gaseous emissions from 28 individual diesel-fuelled and 7 compressed natural gas (CNG-fuelled buses, selected from an in-use bus fleet, were characterised for real-world dilution scenarios. The method used was based on using CO2 as a tracer of exhaust gas dilution. The particles were sampled by using an extractive sampling method and analysed with high time resolution instrumentation EEPS (10 Hz and CO2 with a non-dispersive infrared gas analyser (LI-840, LI-COR Inc. 1 Hz. The gaseous constituents (CO, HC and NO were measured by using a remote sensing device (AccuScan RSD 3000, Environmental System Products Inc.. Nitrogen oxides, NOx, were estimated from NO by using default NO2/NOx ratios from the road vehicle emission model HBEFA3.1. The buses studied were diesel-fuelled Euro III–V and CNG-fuelled Enhanced Environmentally Friendly Vehicles (EEVs with different after-treatment, including selective catalytic reduction (SCR, exhaust gas recirculation (EGR and with and without diesel particulate filter (DPF. The primary driving mode applied in this study was accelerating mode. However, regarding the particle emissions also a constant speed mode was analysed. The investigated CNG buses emitted on average a higher number of particles but less mass compared to the diesel-fuelled buses. Emission factors for number of particles (EFPN were EFPN, DPF = 4.4 ± 3.5 × 1014, EFPN, no DPF = 2.1 ± 1.0 × 1015 and EFPN, CNG = 7.8 ± 5.7 ×1015 kg fuel−1. In the accelerating mode, size-resolved emission factors (EFs showed unimodal number size distributions with peak diameters of 70–90 nm and 10 nm for diesel and CNG buses, respectively. For the constant speed mode, bimodal average number size distributions were obtained for the diesel buses with peak modes of ~10 nm and ~60 nm. Emission factors for NOx expressed as NO2 equivalents for the diesel buses were on average 27 ± 7 g (kg fuel−1 and for the CNG buses 41

The ir emission features: Emission from PAH (Polycyclic Aromatic Hydrocarbons) molecules and amorphous carbon particles

Energy Technology Data Exchange (ETDEWEB)

Allamandola, L.J.; Tielens, A.G.G.M.; Barker, J.R.

1986-01-01

PAHs can have several forms in the interstellar medium. To assess the importance of each requires the availability of a collection of high quality, complete mid-ir interstellar emission spectra, a collection of laboratory spectra of PAH samples prepared under realistic conditions and a firm understanding of the microscopic emission mechanism. Given what we currently know about PAHs, the spectroscopic data suggests that there are at least two components which contribute to the interstellar emission spectrum: free molecule sized PAHs producing the narrow features and amorphous carbon particles (which are primarily made up of an irregular ''lattice'' of PAHs) contributing to the broad underlying components. An exact treatment of the ir fluorescence from highly vibrationally excited large molecules shows that species containing between 20 and 30 carbon atoms are responsible for the narrow features, although the spectra match more closely with the spectra of amorphous carbon particles. Since little is known about the spectroscopic properties of free PAHs and PAH clusters, much laboratory work is called for in conjunction with an observational program which focuses on the spatial characteristics of the spectra. In this way the distribution and evolution of carbon from molecule to particle can be traced. 38 refs., 9 figs.

The ir emission features: Emission from PAH [Polycyclic Aromatic Hydrocarbons] molecules and amorphous carbon particles

International Nuclear Information System (INIS)

Allamandola, L.J.; Tielens, A.G.G.M.; Barker, J.R.

1986-01-01

PAHs can have several forms in the interstellar medium. To assess the importance of each requires the availability of a collection of high quality, complete mid-ir interstellar emission spectra, a collection of laboratory spectra of PAH samples prepared under realistic conditions and a firm understanding of the microscopic emission mechanism. Given what we currently know about PAHs, the spectroscopic data suggests that there are at least two components which contribute to the interstellar emission spectrum: free molecule sized PAHs producing the narrow features and amorphous carbon particles (which are primarily made up of an irregular ''lattice'' of PAHs) contributing to the broad underlying components. An exact treatment of the ir fluorescence from highly vibrationally excited large molecules shows that species containing between 20 and 30 carbon atoms are responsible for the narrow features, although the spectra match more closely with the spectra of amorphous carbon particles. Since little is known about the spectroscopic properties of free PAHs and PAH clusters, much laboratory work is called for in conjunction with an observational program which focuses on the spatial characteristics of the spectra. In this way the distribution and evolution of carbon from molecule to particle can be traced. 38 refs., 9 figs

Density and energy distribution of epithermal secondary electrons in a plasma with fast charged particles

International Nuclear Information System (INIS)

Jayakumar, R.; Fleischmann, H.H.

1989-01-01

The production of intermediate energy secondary electrons in plasmas through collisions with fast charged particles is investigated. The density and the distribution of the secondary electrons are obtained by calculating the generation, slow down and diffusion rates, using basic Rutherford collision cross sections. It is shown that the total density of secondaries is much smaller than the fast particle density and that the energy distribution has roughly a 1/√E dependence. The higher generation secondary populations are also obtained. (orig.)

Test Method for High β Particle Emission Rate of 63Ni Source Plate

OpenAIRE

ZHANG Li-feng

2015-01-01

For the problem of measurement difficulties of β particle emission rate of Ni-63 source plate used for Ni-63 betavoltaic battery, a relative test method of scintillation current method was erected according to the measurement principle of scintillation detector.β particle emission rate of homemade Ni-63 source plate was tested by the method, and the test results were analysed and evaluated, it was initially thought that scintillation current method was a feasible way of testing β particle emi...

Isoprene in poplar emissions: effects on new particle formation and OH concentrations

Science.gov (United States)

Kiendler-Scharr, A.; Andres, S.; Bachner, M.; Behnke, K.; Broch, S.; Hofzumahaus, A.; Holland, F.; Kleist, E.; Mentel, T. F.; Rubach, F.; Springer, M.; Steitz, B.; Tillmann, R.; Wahner, A.; Schnitzler, J.-P.; Wildt, J.

2012-01-01

Stress-induced volatile organic compound (VOC) emissions from transgenic Grey poplar modified in isoprene emission potential were used for the investigation of photochemical secondary organic aerosol (SOA) formation. In poplar, acute ozone stress induces the emission of a wide array of VOCs dominated by sesquiterpenes and aromatic VOCs. Constitutive light-dependent emission of isoprene ranged between 66 nmol m-2 s-1 in non-transgenic controls (wild type WT) and nearly zero (plants (line RA22), respectively. Nucleation rates of up to 3600 cm-3 s-1 were observed in our experiments. In the presence of isoprene new particle formation was suppressed compared to non-isoprene containing VOC mixtures. Compared to isoprene/monoterpene systems emitted from other plants the suppression of nucleation by isoprene was less effective for the VOC mixture emitted from stressed poplar. This is explained by the observed high efficiency of new particle formation for emissions from stressed poplar. Direct measurements of OH in the reaction chamber revealed that the steady state concentration of OH is lower in the presence of isoprene than in the absence of isoprene, supporting the hypothesis that isoprenes' suppressing effect on nucleation is related to radical chemistry. In order to test whether isoprene contributes to SOA mass formation, fully deuterated isoprene (C5D8) was added to the stress-induced emission profile of an isoprene free poplar mutant. Mass spectral analysis showed that, despite the isoprene-induced suppression of particle formation, fractions of deuterated isoprene were incorporated into the SOA. A fractional mass yield of 2.3% of isoprene was observed. Future emission changes due to land use and climate change may therefore affect both gas phase oxidation capacity and new particle number formation.

Intermittent behavior of fast and slow target fragments from 16O-AgBr interactions at 3.7 A GeV

International Nuclear Information System (INIS)

Li Junsheng; Zhang Donghai; Liu Fuhu

2008-01-01

Angular distributions of fast and slow target particles produced in 16 O-AgBr interaction at 3.7 A GeV have been reported. Intermittency and fractal behavior have been studied for emission spectra of target associated fast and slow particles. Intermittent behavior is observed for both knocked out and slow target fragments. In both the cases anomalous dimensions are seen to increase with the order of moments thereby indicating the association of multifractility with production mechanism of both fast and slow target associated particles

A method for measuring particle number emissions from vehicles driving on the road.

Science.gov (United States)

Shi, J P; Harrison, R M; Evans, D E; Alam, A; Barnes, C; Carter, G

2002-01-01

Earlier research has demonstrated that the conditions of dilution of engine exhaust gases profoundly influence the size distribution and total number of particles emitted. Since real world dilution conditions are variable and therefore difficult to simulate, this research has sought to develop and validate a method for measuring particle number emissions from vehicles driving past on a road. This has been achieved successfully using carbon dioxide as a tracer of exhaust gas dilution. By subsequent adjustment of data to a constant dilution factor, it is possible to compare emissions from different vehicles using different technologies and fuels based upon real world emission data. Whilst further optimisation of the technique, especially in terms of matching the instrument response times is desirable, the measurements offer useful insights into emissions from gasoline and diesel vehicles, and the substantial proportion of particles emitted in the 3-7 nanometre size range.

Anisotropic and correlated emissions of short range charged particles in anti pAg/Br reactions of 1.4 GeV/c incident momentum observed in photographic emulsions

International Nuclear Information System (INIS)

Breivik, F.O.; Jacobsen, T.; Soerensen, S.O.

1983-12-01

Anti pAg/Br reactions at 1.4 GeV/c incident momentum were studied by means of the emulsion technique. A group of short range charged particles was observed. For the events with one short track, a backward and transversal emission was seen, probably due to some very fast process. For the events with two short tracks, a back-to-back emission was seen, indicating some two-body decay where the target nucleus possibly behaves spectator-like. The rates and forward collimations suggest that the same physical process causes the different multiplicities

Developing Particle Emission Inventories Using Remote Sensing (PEIRS)

Science.gov (United States)

Tang, Chia-Hsi; Coull, Brent A.; Schwartz, Joel; Lyapustin, Alexei I.; Di, Qian; Koutrakis, Petros

2016-01-01

Information regarding the magnitude and distribution of PM(sub 2.5) emissions is crucial in establishing effective PM regulations and assessing the associated risk to human health and the ecosystem. At present, emission data is obtained from measured or estimated emission factors of various source types. Collecting such information for every known source is costly and time consuming. For this reason, emission inventories are reported periodically and unknown or smaller sources are often omitted or aggregated at large spatial scale. To address these limitations, we have developed and evaluated a novel method that uses remote sensing data to construct spatially-resolved emission inventories for PM(sub 2.5). This approach enables us to account for all sources within a fixed area, which renders source classification unnecessary. We applied this method to predict emissions in the northeast United States during the period of 2002-2013 using high- resolution 1 km x 1 km Aerosol Optical Depth (AOD). Emission estimates moderately agreed with the EPA National Emission Inventory (R(sup2) = 0.66 approx. 0.71, CV = 17.7 approx. 20%). Predicted emissions are found to correlate with land use parameters suggesting that our method can capture emissions from land use-related sources. In addition, we distinguished small-scale intra-urban variation in emissions reflecting distribution of metropolitan sources. In essence, this study demonstrates the great potential of remote sensing data to predict particle source emissions cost-effectively.

Light particle revelation on incomplete fusion reactions

International Nuclear Information System (INIS)

Gillibert, A.

1984-01-01

Incomplete fusion reactions have been studied through light particles emission in the reaction 116 Sn + 16 O at 125 MeV (ALICE facility in Orsay). We measured energy angular distributions and correlations between any two of these particles (α particles, protons, neutrons), while γ multiplicity measurements provide us fuller informations. From collected data, the following pictures can be drawn: - the only fast particles observed are α particles, while protons and neutrons seem to come only from statistical evaporation; - outgoing channels where two α particles are emitted cannot be solely explained by the sequential emission of 8 Be → 2α: about half of the cross section proceeds from statistical evaporation of one α particle. Accordingly, 2αxn channels do not necessarily agree with high value of angular momentum in the entrance channel. From the study of experimental results in the yrast plane, we can assign a large width to the angular momentum distribution [fr

Isoprene in poplar emissions: effects on new particle formation and OH concentrations

Directory of Open Access Journals (Sweden)

A. Kiendler-Scharr

2012-01-01

Full Text Available Stress-induced volatile organic compound (VOC emissions from transgenic Grey poplar modified in isoprene emission potential were used for the investigation of photochemical secondary organic aerosol (SOA formation. In poplar, acute ozone stress induces the emission of a wide array of VOCs dominated by sesquiterpenes and aromatic VOCs. Constitutive light-dependent emission of isoprene ranged between 66 nmol m⁻² s⁻¹ in non-transgenic controls (wild type WT and nearly zero (<0.5 nmol m⁻² s⁻¹ in isoprene emission-repressed plants (line RA22, respectively. Nucleation rates of up to 3600 cm⁻³ s⁻¹ were observed in our experiments. In the presence of isoprene new particle formation was suppressed compared to non-isoprene containing VOC mixtures. Compared to isoprene/monoterpene systems emitted from other plants the suppression of nucleation by isoprene was less effective for the VOC mixture emitted from stressed poplar. This is explained by the observed high efficiency of new particle formation for emissions from stressed poplar. Direct measurements of OH in the reaction chamber revealed that the steady state concentration of OH is lower in the presence of isoprene than in the absence of isoprene, supporting the hypothesis that isoprenes' suppressing effect on nucleation is related to radical chemistry. In order to test whether isoprene contributes to SOA mass formation, fully deuterated isoprene (C₅D₈ was added to the stress-induced emission profile of an isoprene free poplar mutant. Mass spectral analysis showed that, despite the isoprene-induced suppression of particle formation, fractions of deuterated isoprene were incorporated into the SOA. A fractional mass yield of 2.3% of isoprene was observed. Future emission changes due to land use and climate change may therefore affect both gas phase oxidation capacity and new particle number formation.

Emission of high-energy, light particles from intermediate-energy heavy-ion reactions

International Nuclear Information System (INIS)

Ball, J.B.; Auble, R.L.

1982-01-01

One of the early surprises in examining reaction products from heavy ion reactions at 10 MeV/nucleon and above was the large yield of light particles emitted and the high energies to which the spectra of these particles extended. The interpretation of the origin of the high energy light ions has evolved from a picture of projectile excitation and subsequent evaporation to one of pre-equilibrium (or nonequilibrium) emission. The time scale for particle emission has thus moved from one that occurs following the initial collision to one that occurs at the very early stages of the collision. Research at ORNL on this phenomenon is reviewed

Comparison of fission probabilities with emission of long range particles under the action of slow and fast neutrons on various materials; Probabilites comparees de fission avec emission de particules de long parcours pour divers materiaux sous l'action des neutrons lents et rapides

Energy Technology Data Exchange (ETDEWEB)

Netter, F; Faraggi, H; Garin-Bonnet, A; Julien, J; Corge, C [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires; Turkiewicz, J [Institut de Recherches Nucleaire de Varsovie (Poland)

1958-07-01

The authors describe relative cross-section measurements of fission of the isotopes of uranium and plutonium (more particularly {sup 235}U, {sup 238}U, {sup 239}Pu), with emission of long range particles, under the action of neutrons of various energies: thermal neutrons, pile neutrons, neutrons produced with the Van de Graaff accelerator by reaction of protons on tritium. The measurements are carried out: 1) with the aid of photographic plates, by submitting to the action of the neutrons a layer of fissile material coupled with an Ilford nuclear emulsion of 200 microns; a tin sheet laying between the plate and the layer stops the {alpha} particles and the fission fragments. By an appropriate development the tracks of the long range particles can be distinguished in the emulsion, from the tracks of the recoil protons resulting of fission neutrons, or of the last primary neutrons. For neutrons of energy under 1 MeV, the compared frequency of the tracks of long range particles and of the recoils caused by the fission neutrons gives a measurement of the fission cross-section with emission of long range particles relative to the product of the fission cross-section by the mean number of neutrons emitted by fission. For neutrons of higher energy, one measures only the frequency of the tracks of long range particles, comparatively with the flux of primary neutrons. Some precautions are taken to eliminate the action of thermal neutrons in the measurements with fast neutrons. 2) with the aid of a system of ionization chamber and proportional counter, the rate of coincidence between the impulsions caused by the long range particles and the impulsions provided by one of the fission fragments is measured comparatively with the counting rate of fission fragme (author) [French] Les auteurs decrivent des mesures relatives a la section efficace de fission des isotopes de l'uranium et du plutonium (notamment {sup 235}U, {sup 238}U, {sup 239}Pu) avec emission de particules de long

A feature point identification method for positron emission particle tracking with multiple tracers

Energy Technology Data Exchange (ETDEWEB)

Wiggins, Cody, E-mail: cwiggin2@vols.utk.edu [University of Tennessee-Knoxville, Department of Physics and Astronomy, 1408 Circle Drive, Knoxville, TN 37996 (United States); Santos, Roque [University of Tennessee-Knoxville, Department of Nuclear Engineering (United States); Escuela Politécnica Nacional, Departamento de Ciencias Nucleares (Ecuador); Ruggles, Arthur [University of Tennessee-Knoxville, Department of Nuclear Engineering (United States)

2017-01-21

A novel detection algorithm for Positron Emission Particle Tracking (PEPT) with multiple tracers based on optical feature point identification (FPI) methods is presented. This new method, the FPI method, is compared to a previous multiple PEPT method via analyses of experimental and simulated data. The FPI method outperforms the older method in cases of large particle numbers and fine time resolution. Simulated data show the FPI method to be capable of identifying 100 particles at 0.5 mm average spatial error. Detection error is seen to vary with the inverse square root of the number of lines of response (LORs) used for detection and increases as particle separation decreases. - Highlights: • A new approach to positron emission particle tracking is presented. • Using optical feature point identification analogs, multiple particle tracking is achieved. • Method is compared to previous multiple particle method. • Accuracy and applicability of method is explored.

Time-resolved analysis of particle emissions from residential biomass combustion - Emissions of refractory black carbon, PAHs and organic tracers

Science.gov (United States)

Nielsen, Ingeborg E.; Eriksson, Axel C.; Lindgren, Robert; Martinsson, Johan; Nyström, Robin; Nordin, Erik Z.; Sadiktsis, Ioannis; Boman, Christoffer; Nøjgaard, Jacob K.; Pagels, Joakim

2017-09-01

Time-resolved particle emissions from a conventional wood stove were investigated with aerosol mass spectrometry to provide links between combustion conditions, emission factors, mixing state of refractory black carbon and implications for organic tracer methods. The addition of a new batch of fuel results in low temperature pyrolysis as the fuel heats up, resulting in strong, short-lived, variable emission peaks of organic aerosol-containing markers of anhydrous sugars, such as levoglucosan (fragment at m/z 60). Flaming combustion results in emissions dominated by refractory black carbon co-emitted with minor fractions of organic aerosol and markers of anhydrous sugars. Full cycle emissions are an external mixture of larger organic aerosol-dominated and smaller thinly coated refractory black carbon particles. A very high burn rate results in increased full cycle mass emission factors of 66, 2.7, 2.8 and 1.3 for particulate polycyclic aromatic hydrocarbons, refractory black carbon, total organic aerosol and m/z 60, respectively, compared to nominal burn rate. Polycyclic aromatic hydrocarbons are primarily associated with refractory black carbon-containing particles. We hypothesize that at very high burn rates, the central parts of the combustion zone become air starved, leading to a locally reduced combustion temperature that reduces the conversion rates from polycyclic aromatic hydrocarbons to refractory black carbon. This facilitates a strong increase of polycyclic aromatic hydrocarbons emissions. At nominal burn rates, full cycle emissions based on m/z 60 correlate well with organic aerosol, refractory black carbon and particulate matter. However, at higher burn rates, m/z 60 does not correlate with increased emissions of polycyclic aromatic hydrocarbons, refractory black carbon and organic aerosol in the flaming phase. The new knowledge can be used to advance source apportionment studies, reduce emissions of genotoxic compounds and model the climate impacts of

Charged particle accelerator

Energy Technology Data Exchange (ETDEWEB)

Ress, T I; Nolde, G V

1974-11-25

A charged particle accelerator is described. It is made of an enclosure arranged for channeling a stream of charged particles along a predetermined path, and propelling means juxtaposed to the enclosure for generating a magnetic field moving in a predetermined direction with respect to each point of the path, the magnetic flux vector of that field being transverse to that path at every point, which gives the particles, along said path, a velocity connected to that of the mobile field by a predetermined relation. This can be applied to the fast production of chemical compounds, to the emission of neutrons and of thermal energy, and to the production of mechanical energy for propelling space ships.

Charged particle accelerator

International Nuclear Information System (INIS)

Ress, T.I.; Nolde, G.V.

1974-01-01

A charged particle accelerator is described. It is made of an enclosure arranged for channeling a stream of charged particles along a predetermined path, and propelling means juxtaposed to said enclosure for generating therein a magnetic field moving in a predetermined direction with respect to each point of said path, the magnetic flux vector of that field being transverse to that path at every point, which gives the particles, along said path, a velocity connected to that of the mobile field by a predetermined relation. This can be applied to the fast production of chemical compounds, to the emission of neutrons and of thermal energy, and to the production of mechanical energy for propelling space ships [fr

Fast Radio Bursts with Extended Gamma-Ray Emission?

International Nuclear Information System (INIS)

Murase, Kohta; Mészáros, Peter; Fox, Derek B.

2017-01-01

We consider some general implications of bright γ -ray counterparts to fast radio bursts (FRBs). We show that even if these manifest in only a fraction of FRBs, γ -ray detections with current satellites (including Swift ) can provide stringent constraints on cosmological FRB models. If the energy is drawn from the magnetic energy of a compact object such as a magnetized neutron star, the sources should be nearby and be very rare. If the intergalactic medium is responsible for the observed dispersion measure, the required γ -ray energy is comparable to that of the early afterglow or extended emission of short γ -ray bursts. While this can be reconciled with the rotation energy of compact objects, as expected in many merger scenarios, the prompt outflow that yields the γ -rays is too dense for radio waves to escape. Highly relativistic winds launched in a precursor phase, and forming a wind bubble, may avoid the scattering and absorption limits and could yield FRB emission. Largely independent of source models, we show that detectable radio afterglow emission from γ -ray bright FRBs can reasonably be anticipated. Gravitational wave searches can also be expected to provide useful tests.

A PEMS study of the emissions of gaseous pollutants and ultrafine particles from gasoline- and diesel-fueled vehicles

Science.gov (United States)

Huang, Cheng; Lou, Diming; Hu, Zhiyuan; Feng, Qian; Chen, Yiran; Chen, Changhong; Tan, Piqiang; Yao, Di

2013-10-01

On-road emission measurements of gasoline- and diesel-fueled vehicles were conducted by a portable emission measurement system (PEMS) in Shanghai, China. Horiba OBS 2200 and TSI EEPS 3090 were employed to detect gaseous and ultrafine particle emissions during the tests. The driving-based emission factors of gaseous pollutants and particle mass and number were obtained on various road types. The average NOx emission factors of the diesel bus, diesel car, and gasoline car were 8.86, 0.68, and 0.17 g km-1, all of which were in excess of their emission limits. The particle number emission factors were 7.06 × 1014, 6.08 × 1014, and 1.57 × 1014 km-1, generally higher than the results for similar vehicle types reported in the previous studies. The size distributions of the particles emitted from the diesel vehicles were mainly concentrated in the accumulation mode, while those emitted from the gasoline car were mainly distributed in the nucleation mode. Both gaseous and particle emission rates exhibit significant correlations with the change in vehicle speed and power demand. The lowest emission rates for each vehicle type were produced during idling. The highest emission rates for each vehicle type were generally found in high-VSP bins. The particle number emission rates of the gasoline car show the strongest growth trend with increasing VSP and speed. The particle number emission for the gasoline car increased by 3 orders of magnitude from idling to the highest VSP and driving speed conditions. High engine power caused by aggressive driving or heavy loads is the main contributor to high emissions for these vehicles in real-world situations.

[Analysis on oil fume particles in catering industry cooking emission].

Science.gov (United States)

Tan, De-Sheng; Kuang, Yuan-Cheng; Liu, Xin; Dai, Fei-Hong

2012-06-01

By measuring the particulate matter of oil fume which is over 10 microm or below 10 microm separately and using microradiography and Electrical Low Pressure Impactor (ELPI), it is found out the distributing characteristic of oil fume particles in catering industry cooking emission. The result shows that the diameter of the oil fume particles which was sedimentated in the kitchen is between 10-400 microm, the concentration peak value is between 10-100 microm. The diameter of oil fume aerosol is mostly smaller than 1 microm, while the concentration peak value is between 0.063-0.109 microm. In addition, the mass concentration peak value is between 6.560-9.990 microm. Through the analysis to the physical characteristics of oil fume from catering industry cooking emissions, the eigenvalue of the oil fume has been found and the feature matter for monitoring the oil fume has been discovered to provide a reasonable standard for controlling and monitoring the catering industry cooking emission.

Self ordering threshold and superradiant backscattering to slow a fast gas beam in a ring cavity with counter propagating pump.

Science.gov (United States)

Maes, C; Asbóth, J K; Ritsch, H

2007-05-14

We study the dynamics of a fast gaseous beam in a high Q ring cavity counter propagating a strong pump laser with large detuning from any particle optical resonance. As spontaneous emission is strongly suppressed the particles can be treated as polarizable point masses forming a dynamic moving mirror. Above a threshold intensity the particles exhibit spatial periodic ordering enhancing collective coherent backscattering which decelerates the beam. Based on a linear stability analysis in their accelerated rest frame we derive analytic bounds for the intensity threshold of this selforganization as a function of particle number, average velocity, kinetic temperature, pump detuning and resonator linewidth. The analytical results agree well with time dependent simulations of the N-particle motion including field damping and spontaneous emission noise. Our results give conditions which may be easily evaluated for stopping and cooling a fast molecular beam.

A model for particle emission from a fissioning system

International Nuclear Information System (INIS)

Milek, B.; Reif, R.; Revai, J.

1987-04-01

The differential emission probability for a neutron emitted in a binary fission process due to non-adiabatic effects in the coupling of the single particle degrees of freedom to the accelerated relative motion of the fragments is investigated wihtin a model, which represents each nucleus by a non-deformed one-term separable potential. The derivation of measurable quantities from the asymptotic solution of the time-dependent Schroedinger equation for the single particle wave function is examined. Numerical calculations were performed for parameter values, which correspond to 252 Cf(sf). The calculated energy spectra and angular distributions of the emitted particles are presented in dependence on the mass asymmetry. (author)

The pick-up mechanism in composite particle emission processes

International Nuclear Information System (INIS)

Zhang Jingshang; Yan Shiwei; Wang Cuilan

1992-01-01

The pick-up mechanism has been included in the exciton model for the light composite particle emissions. Based on the cluster phase space integration method the formation probabilities of α,d,t, 3 He are obtained. The calculation results of (n,t) cross sections indicate that this theoretical method can reproduce the experimental data nicely. For triton emissions in pre-equilibrium reaction processes, the semi-direct reactions are the dominant terms which are just omitted in the previous model calculation

Light-particle emission and heavy residues from nucleus-nucleus collisions

International Nuclear Information System (INIS)

Caplar, R.; Hoelbling, S.; Gentner, R.; Lassen, L.; Oberstedt, A.

1991-01-01

We have investigated the interrelation between light-particle multiplicities and mass resp. charge distributions of heavy residues from complete and incomplete fusion of heavy ions. We have shown that a simple statistical model provides the possibility of quantitatively correlating heavy-residue distributions and corresponding light-particle multiplicities both at the Coulomb barrier and at higher energies where preequilibrium emission occurs. (author). 8 refs, 4 figs, 1 tab

Fast weighted centroid algorithm for single particle localization near the information limit.

Science.gov (United States)

Fish, Jeremie; Scrimgeour, Jan

2015-07-10

A simple weighting scheme that enhances the localization precision of center of mass calculations for radially symmetric intensity distributions is presented. The algorithm effectively removes the biasing that is common in such center of mass calculations. Localization precision compares favorably with other localization algorithms used in super-resolution microscopy and particle tracking, while significantly reducing the processing time and memory usage. We expect that the algorithm presented will be of significant utility when fast computationally lightweight particle localization or tracking is desired.

A fast iterative method for computing particle beams penetrating matter

International Nuclear Information System (INIS)

Boergers, C.

1997-01-01

Beams of microscopic particles penetrating matter are important in several fields. The application motivating our parameter choices in this paper is electron beam cancer therapy. Mathematically, a steady particle beam penetrating matter, or a configuration of several such beams, is modeled by a boundary value problem for a Boltzmann equation. Grid-based discretization of this problem leads to a system of algebraic equations. This system is typically very large because of the large number of independent variables in the Boltzmann equation (six if time independence is the only dimension-reducing assumption). If grid-based methods are to be practical at all, it is therefore necessary to develop fast solvers for the discretized problems. This is the subject of the present paper. For two-dimensional, mono-energetic, linear particle beam problems, we describe an iterative domain decomposition algorithm based on overlapping decompositions of the set of particle directions and computationally demonstrate its rapid, grid independent convergence. There appears to be no fundamental obstacle to generalizing the method to three-dimensional, energy dependent problems. 34 refs., 15 figs., 6 tabs

Challenges and Approaches for Developing Ultrafine Particle Emission Inventories for Motor Vehicle and Bus Fleets

Directory of Open Access Journals (Sweden)

Diane U. Keogh

2011-03-01

Full Text Available Motor vehicles in urban areas are the main source of ultrafine particles (diameters < 0.1 µm. Ultrafine particles are generally measured in terms of particle number because they have little mass and are prolific in terms of their numbers. These sized particles are of particular interest because of their ability to enter deep into the human respiratory system and contribute to negative health effects. Currently ultrafine particles are neither regularly monitored nor regulated by ambient air quality standards. Motor vehicle and bus fleet inventories, epidemiological studies and studies of the chemical composition of ultrafine particles are urgently needed to inform scientific debate and guide development of air quality standards and regulation to control this important pollution source. This article discusses some of the many challenges associated with modelling and quantifying ultrafine particle concentrations and emission rates for developing inventories and microscale modelling of motor vehicles and buses, including the challenge of understanding and quantifying secondary particle formation. Recommendations are made concerning the application of particle emission factors in developing ultrafine particle inventories for motor vehicle fleets. The article presents a précis of the first published inventory of ultrafine particles (particle number developed for the urban South-East Queensland motor vehicle and bus fleet in Australia, and comments on the applicability of the comprehensive set of average particle emission factors used in this inventory, for developing ultrafine particle (particle number and particle mass inventories in other developed countries.

Dirac Particles Emission from An Elliptical Black Hole

Directory of Open Access Journals (Sweden)

Yuant Tiandho

2017-03-01

Full Text Available According to the general theory of relativiy, a black hole is defined as a region of spacetime with super-strong gravitational effects and there is nothing can escape from it. So in the classical theory of relativity, it is safe to say that black hole is a "dead" thermodynamical object. However, by using quantum mechanics theory, Hawking has shown that a black hole may emit particles. In this paper, calculation of temperature of an elliptical black hole when emitting the Dirac particles was presented. By using the complexpath method, radiation can be described as emission process in the tunneling pictures. According to relationship between probability of outgoing particle with the spectrum of black body radiation for fermion particles, temperature of the elliptical black hole can be obtained and it depend on the azimuthal angle. This result also showed that condition on the surface of elliptical black hole is not in thermal equilibrium.

Solar energetic particles and radio burst emission

Directory of Open Access Journals (Sweden)

Miteva Rositsa

2017-01-01

Full Text Available We present a statistical study on the observed solar radio burst emission associated with the origin of in situ detected solar energetic particles. Several proton event catalogs in the period 1996–2016 are used. At the time of appearance of the particle origin (flare and coronal mass ejection we identified radio burst signatures of types II, III and IV by inspecting dynamic radio spectral plots. The information from observatory reports is also accounted for during the analysis. The occurrence of solar radio burst signatures is evaluated within selected wavelength ranges during the solar cycle 23 and the ongoing 24. Finally, we present the burst occurrence trends with respect to the intensity of the proton events and the location of their solar origin.

Proposed neutral-beam diagnostics for fast confined alpha particles in a burning plasma

International Nuclear Information System (INIS)

Schlachter, A.S.; Cooper, W.S.

1986-10-01

Diagnostic methods for fast confined alpha particles are essential for a burning plasma experiment. Several methods which use energetic neutral beams have been proposed. We review these methods and discuss system considerations for their implementation

Housing and sustainable development: perspectives offered by thermal solar energy. Particle emissions: prospective investigation of primary particle emissions in France by 2030

International Nuclear Information System (INIS)

Brignon, J.M.; Cauret, L.; Sambat, S.

2004-09-01

This publication proposes two investigation reports. A first study proposes a prospective analysis of the housing 'stock' in France and the evolution of global energy consumptions and CO 2 emissions by the housing sector, a prospective study of space heating and hot water needs by defining reference scenarios as well as a target scenario for heating consumption (based on the factor 4 of reduction of emissions by 2050), and an assessment of the contribution of the thermal solar energy applied to winter comfort under the form of direct solar floors and passive solar contributions, and applied to hot water by 2050. The contribution of the thermal solar energy is studied within its regulatory context. An analysis of urban forms is also performed to assess the potential of integration of renewable energy solutions in the existing housing stock, and thus to assess the morphological limits of an attempt of generalized solarization of roofs. The second study proposes a detailed identification and assessment of the various sources of primary particles (combustion, industrial processes, mineral extraction and processing, road transport, waste processing and elimination, agriculture, natural sources, forest fires), providing more precise results and methodological complements for some sources. It also proposes a prospective assessment of emissions and identifies the main factors of particle concentrations in urban environment

Ultrafine particle emissions by in-use diesel buses of various generations at low-load regimes

Science.gov (United States)

Tartakovsky, L.; Baibikov, V.; Comte, P.; Czerwinski, J.; Mayer, A.; Veinblat, M.; Zimmerli, Y.

2015-04-01

Ultrafine particles (UFP) are major contributors to air pollution due to their easy gas-like penetration into the human organism, causing adverse health effects. This study analyzes UFP emissions by buses of different technologies (from Euro II till Euro V EEV - Enhanced Environmentally-friendly Vehicle) at low-load regimes. Additionally, the emission-reduction potential of retrofitting with a diesel particle filter (DPF) is demonstrated. A comparison of the measured, engine-out, particle number concentrations (PNC) for buses of different technological generations shows that no substantial reduction of engine-out emissions at low-load operating modes is observed for newer bus generations. Retrofitting the in-use urban and interurban buses of Euro II till Euro IV technologies by the VERT-certified DPF confirmed its high efficiency in reduction of UFP emissions. Particle-count filtration efficiency values of the retrofit DPF were found to be extremely high - greater than 99.8%, similar to that of the OEM filter in the Euro V bus.

Investigation of granular impact using positron emission particle tracking

KAUST Repository

Marston, Jeremy O.

2015-04-01

We present results from an experimental study of granular impact using a combination of high-speed video and positron emission particle tracking (PEPT). The PEPT technique exploits the annihilation of photons from positron decay to determine the position of tracer particles either inside a small granular bed or attached to the object which impacts the bed. We use dense spheres as impactors and the granular beds are comprised of glass beads which are fluidised to achieve a range of different initial packing states. For the first time, we have simultaneously investigated both the trajectory of the sphere, the motion of particles in a 3-D granular bed and particles which jump into the resultant jet, which arises from the collapse of the cavity formed by the impacting sphere.

Fast imaging measurements and modeling of neutral and impurity density on C-2U

Science.gov (United States)

Granstedt, Erik; Deng, B.; Dettrick, S.; Gupta, D. K.; Osin, D.; Roche, T.; Zhai, K.; TAE Team

2016-10-01

The C-2U device employed neutral beam injection and end-biasing to sustain an advanced beam-driven Field-Reversed Configuration plasma for 5+ ms, beyond characteristic transport time-scales. Three high-speed, filtered cameras observed visible light emission from neutral hydrogen and impurities, as well as deuterium pellet ablation and compact-toroid injection which were used for auxiliary particle fueling. Careful vacuum practices and titanium gettering successfully reduced neutral recycling from the confinement vessel wall. As a result, a large fraction of the remaining neutrals originate from charge-exchange between the neutral beams and plasma ions. Measured H/D- α emission is used with DEGAS2 neutral particle modeling to reconstruct the strongly non-axissymmetric neutral distribution. This is then used in fast-ion modeling to more accurately estimate their charge-exchange loss rate. Oxygen emission due to electron-impact excitation and charge-exchange recombination has also been measured using fast imaging. Reconstructed emissivity of O4+ is localized on the outboard side of the core plasma near the estimated location of the separatrix inferred by external magnetic measurements. Tri Alpha Energy.

Light particle emission measurements in heavy ion reactions: Progress report, June 1, 1988--May 31, 1989

International Nuclear Information System (INIS)

Petitt, G.A.

1989-01-01

We have completed another successful year of experimental work at the Heavy Ion Research Facility (HHIRF) and at Georgia State University (GSU). Since submitting our previous progress report we have completed our paper on neutron emission from products of the reaction 58 Ni + 165 Ho and it has been submitted to Physical Review C. Some of the details of these results are discussed below. We have installed the Vaxstation computer system for which we received supplemental funding from DOE during 1988-89 and it is being used to analyze the Ni + Ho data using the codes Pace and a modified version of Lilita, both of which we have been able to transfer to our Vaxstation systems from the Vax at ORNL with very minimal modification. The Exabyte tape drive which we ordered with the computer system was finally delivered at the end of January after months of delays. It is now being used to scan data tapes from our experiment to study neutron-neutron and neutron-charged-particle momentum correlations using the reaction 32 S + 197 Au at 25 MeV/nucleon. This data analysis can now proceed at a fast pace. Finally, we have continued our developmental work on the Hili detector system at ORNL, and have participated in experiments to study the predictions of the Dyabatic Dynamics model of particle emission using the Ni + Ni system and the HILI detector system

Ion cyclotron emission by spontaneous emission

Energy Technology Data Exchange (ETDEWEB)

Da Costa, O [Commission of the European Communities, Abingdon (United Kingdom). JET Joint Undertaking; Gresillon, D [Ecole Polytechnique, 91 - Palaiseau (France). Lab. de Physique des Milieux Ionises

1994-07-01

The goal of the study is to examine whether the spontaneous emission can account for ICE (ion cyclotron emission) experimental results, or part of them. A straightforward approach to plasma emission is chosen, investigating the near equilibrium wave radiation by gyrating ions, and thus building from the majority and fast fusion ions the plasma fluctuations and emission on the fast magnetoacoustic or compressional Alfven wave mode in the IC frequency range. Similarities with the ICE experiments are shown: the emission temperature in the presence of fast ions (even in a very small amount), the strong fast ion emission increase with the harmonic, the fine double-line splitting of each peak, the linear but not proportional increase of the peak width with the harmonic. 3 refs., 2 figs.

Ion cyclotron emission by spontaneous emission

International Nuclear Information System (INIS)

Da Costa, O.; Gresillon, D.

1994-01-01

The goal of the study is to examine whether the spontaneous emission can account for ICE (ion cyclotron emission) experimental results, or part of them. A straightforward approach to plasma emission is chosen, investigating the near equilibrium wave radiation by gyrating ions, and thus building from the majority and fast fusion ions the plasma fluctuations and emission on the fast magnetoacoustic or compressional Alfven wave mode in the IC frequency range. Similarities with the ICE experiments are shown: the emission temperature in the presence of fast ions (even in a very small amount), the strong fast ion emission increase with the harmonic, the fine double-line splitting of each peak, the linear but not proportional increase of the peak width with the harmonic. 3 refs., 2 figs

Influence of complex particle emission on properties of giant dipole resonance of hot nuclei

International Nuclear Information System (INIS)

Wen Wanxin; Jin Genming

2003-01-01

The possible reasons for the discrepancy between calculation results based on the statistical evaporation model and experimental data of giant dipole resonance of very hot nuclei are discussed. Both of simulations with the standard CASCADE code and the code coupling complex particle emission are carried out. It is shown that the complex particle emission affects the properties of giant dipole resonance of very hot nuclei

Individual metal-bearing particles in a regional haze caused by firecracker and firework emissions

Energy Technology Data Exchange (ETDEWEB)

Li, Weijun [Environment Research Institute, Shandong University, Jinan, Shandong 250100 (China); State Key of Laboratory of Atmospheric Boundary Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029 (China); Shi, Zongbo [School of Geography, Earth and Environmental Sciences, University of Birmingham (United Kingdom); Yan, Chao; Yang, Lingxiao; Dong, Can; Wang, Wenxing [Environment Research Institute, Shandong University, Jinan, Shandong 250100 (China)

2013-01-15

Intensive firecracker/firework displays during Chinese New Year (CNY) release fine particles and gaseous pollutants into the atmosphere, which may lead to serious air pollution. We monitored ambient PM{sub 2.5} and black carbon (BC) concentrations at a regional background site in the Yellow River Delta region during the CNY in 2011. Our monitoring data and MOUDI images showed that there was a haze event during the CNY. Daily average PM{sub 2.5} concentration reached 183 μg m{sup −3} during the CNY, which was six times higher than that before and after the CNY. Similarly, the black carbon (BC) concentrations were elevated during the CNY. In order to confirm whether the firecracker/firework related emission is the main source of the haze particles, we further analyzed the morphology and chemical composition of individual airborne particles collected before, during and after the CNY by using transmission electron microscopy coupled with energy-dispersive X-ray spectroscopy (TEM/EDS). We found that sulfate and organic-rich particles were dominant in the atmosphere before and after the CNY. In contrast, K-rich sulfates and other metal (e.g., Ba-rich, Al-rich, Mg-rich, and Fe-rich) particles were much more abundant than ammoniated sulfate particles during the CNY. These data suggest that it was the aerosol particles from the firecracker/firework emissions that induced the regional haze episode during the CNY. In individual organic and K-rich particles, we often found more than two types of nano-metal particles. These metal-bearing particles also contained abundant S but not Cl. In contrast, fresh metal-bearing particles from firecrackers generated in the laboratory contained abundant Cl with minor amounts of S. This indicates that the firecracker/firework emissions during the CNY significantly changed the atmospheric transformation pathway of SO{sub 2} to sulfate. - Highlights: ► TEM was used to observe the aged individual particles from firecrackers

Individual metal-bearing particles in a regional haze caused by firecracker and firework emissions

International Nuclear Information System (INIS)

Li, Weijun; Shi, Zongbo; Yan, Chao; Yang, Lingxiao; Dong, Can; Wang, Wenxing

2013-01-01

Intensive firecracker/firework displays during Chinese New Year (CNY) release fine particles and gaseous pollutants into the atmosphere, which may lead to serious air pollution. We monitored ambient PM 2.5 and black carbon (BC) concentrations at a regional background site in the Yellow River Delta region during the CNY in 2011. Our monitoring data and MOUDI images showed that there was a haze event during the CNY. Daily average PM 2.5 concentration reached 183 μg m −3 during the CNY, which was six times higher than that before and after the CNY. Similarly, the black carbon (BC) concentrations were elevated during the CNY. In order to confirm whether the firecracker/firework related emission is the main source of the haze particles, we further analyzed the morphology and chemical composition of individual airborne particles collected before, during and after the CNY by using transmission electron microscopy coupled with energy-dispersive X-ray spectroscopy (TEM/EDS). We found that sulfate and organic-rich particles were dominant in the atmosphere before and after the CNY. In contrast, K-rich sulfates and other metal (e.g., Ba-rich, Al-rich, Mg-rich, and Fe-rich) particles were much more abundant than ammoniated sulfate particles during the CNY. These data suggest that it was the aerosol particles from the firecracker/firework emissions that induced the regional haze episode during the CNY. In individual organic and K-rich particles, we often found more than two types of nano-metal particles. These metal-bearing particles also contained abundant S but not Cl. In contrast, fresh metal-bearing particles from firecrackers generated in the laboratory contained abundant Cl with minor amounts of S. This indicates that the firecracker/firework emissions during the CNY significantly changed the atmospheric transformation pathway of SO 2 to sulfate. - Highlights: ► TEM was used to observe the aged individual particles from firecrackers/fireworks during the Chinese New

High spatio-temporal resolution pollutant measurements of on-board vehicle emissions using ultra-fast response gas analyzers

Directory of Open Access Journals (Sweden)

M. Irwin

2018-06-01

Full Text Available Existing ultra-fast response engine exhaust emissions analyzers have been adapted for on-board vehicle use combined with GPS data. We present, for the first time, how high spatio-temporal resolution data products allow transient features associated with internal combustion engines to be examined in detail during on-road driving. Such data are both useful to examine the circumstances leading to high emissions, and reveals the accurate position of urban air quality hot spots as deposited by the candidate vehicle, useful for source attribution and dispersion modelling. The fast response time of the analyzers, which results in 100 Hz data, makes accurate time-alignment with the vehicle's engine control unit (ECU signals possible. This enables correlation with transient air fuel ratio, engine speed, load, and other engine parameters, which helps to explain the causes of the emissions spikes that portable emissions measurement systems (PEMS and conventional slow response analyzers would miss or smooth out due to mixing within their sampling systems. The data presented is from NO and NOx analyzers, but other fast analyzers (e.g. total hydrocarbons (THC, CO and CO2 can be used similarly. The high levels of NOx pollution associated with accelerating on entry ramps to motorways, driving over speed bumps, accelerating away from traffic lights, are explored in detail. The time-aligned ultra-fast analyzers offer unique insight allowing more accurate quantification and better interpretation of engine and driver activity and the associated emissions impact on local air quality.

Solar energetic particles and radio burst emission

Czech Academy of Sciences Publication Activity Database

Miteva, R.; Samwel, S. W.; Krupař, Vratislav

2017-01-01

Roč. 7 (2017), č. článku A37. ISSN 2115-7251 R&D Projects: GA ČR(CZ) GJ17-06818Y Institutional support: RVO:68378289 Keywords : solar energetic particles * solar radio burst emission * solar cycle Subject RIV: BL - Plasma and Gas Discharge Physics OBOR OECD: Fluids and plasma physics (including surface physics) Impact factor: 2.446, year: 2016 https://www.swsc-journal.org/ articles /swsc/abs/2017/01/swsc170028/swsc170028.html

Influence of suspended particles on the emission of organophosphate flame retardant from insulation boards.

Science.gov (United States)

Lazarov, Borislav; Swinnen, Rudi; Poelmans, David; Spruyt, Maarten; Goelen, Eddy; Covaci, Adrian; Stranger, Marianne

2016-09-01

The influence of the presence of the so-called seed particles on the emission rate of Tris (1-chloroisopropyl) phosphate (TCIPP) from polyisocyanurate (PIR) insulation boards was investigated in this study. Two Field and Laboratory Emission Test cells (FLEC) were placed on the surface of the same PIR board and respectively supplied with clean air (reference FLEC) and air containing laboratory-generated soot particles (test FLEC). The behavior of the area-specific emission rates (SER A ) over a time period of 10 days was studied by measuring the total (gas + particles) concentrations of TCIPP at the exhaust of each FLEC. The estimated SER A of TCIPP from the PIR board at the quasi-static equilibrium were found to be 0.82 μg m(-2) h(-1) in the absence of seed particles, while the addition of soot particles led to SER A of 2.16 μg m(-2) h(-1). This indicates an increase of the SER A of TCIPP from the PIR board with a factor of 3 in the presence of soot particles. The TCIPP partition coefficient to soot particles at the quasi-static equilibrium was 0.022 ± 0.012 m(3) μg(-1). In the next step, the influence of real-life particles on TCIPP emission rates was investigated by supplying the test FLEC with air from a professional kitchen where mainly frying and baking activities took place. Similar to the reference FLEC outcomes, SER A was also found to increase in this real-life experiment over a time period of 20 days by a factor 3 in the presence of particles generated during cooking activities. The median value of estimated particle-gas coefficient for this test was 0.062 ± 0.037 m(3) μg(-1).

A Thomson scattering diagnostic to measure fast ion and α-particle distributions in JET

International Nuclear Information System (INIS)

Costley, A.E.; Hoekzema, J.A.; Stott, P.E.; Watkins, M.L.

1988-01-01

The paper presents the findings of a feasibility investigation into the proposed Thomson scattering diagnostic to measure fast ion and α-particle distributions in JET. A description is given of the motivation for alpha particle diagnostics on JET, followed by a brief survey of possible α-particle diagnostics for JET. The basic principles of the collective Thomson scattering technique are presented, along with its implementation on JET. The expected performance of the system, and other applications of the diagnostic system are also discussed. (U.K.)

General decay law for emission of charged particles and exotic cluster radioactivity

International Nuclear Information System (INIS)

Sahu, Basudeb; Paira, Ramkrishna; Rath, Biswanath

2013-01-01

For the emission of charged particles from metastable nuclei, a general decay formula is developed based on the basic phenomenon of resonances occurring in quantum scattering process under Coulomb-nuclear potential. It relates the half-lives of monopole radioactive decays with the Q-values of the outgoing elements in different angular momentum states as well as the masses and charges of the nuclei involved in the decay. The relation is found to be a generalization of the Geiger–Nuttall law in α radioactivity and it explains well all known emission of charged particles including clusters, alpha and proton carrying angular momenta

Fast Emission Estimates in China Constrained by Satellite Observations (Invited)

Science.gov (United States)

Mijling, B.; van der A, R.

2013-12-01

Emission inventories of air pollutants are crucial information for policy makers and form important input data for air quality models. Unfortunately, bottom-up emission inventories, compiled from large quantities of statistical data, are easily outdated for an emerging economy such as China, where rapid economic growth changes emissions accordingly. Alternatively, top-down emission estimates from satellite observations of air constituents have important advantages of being spatial consistent, having high temporal resolution, and enabling emission updates shortly after the satellite data become available. Constraining emissions from concentration measurements is, however, computationally challenging. Within the GlobEmission project of the European Space Agency (ESA) a new algorithm has been developed, specifically designed for fast daily emission estimates of short-lived atmospheric species on a mesoscopic scale (0.25 × 0.25 degree) from satellite observations of column concentrations. The algorithm needs only one forward model run from a chemical transport model to calculate the sensitivity of concentration to emission, using trajectory analysis to account for transport away from the source. By using a Kalman filter in the inverse step, optimal use of the a priori knowledge and the newly observed data is made. We apply the algorithm for NOx emission estimates in East China, using the CHIMERE model together with tropospheric NO2 column retrievals of the OMI and GOME-2 satellite instruments. The observations are used to construct a monthly emission time series, which reveal important emission trends such as the emission reduction measures during the Beijing Olympic Games, and the impact and recovery from the global economic crisis. The algorithm is also able to detect emerging sources (e.g. new power plants) and improve emission information for areas where proxy data are not or badly known (e.g. shipping emissions). The new emission estimates result in a better

Comparison Between Weisskopf and Thomas-Fermi Model for Particle Emission Widths from Hot Deformed Nuclei

International Nuclear Information System (INIS)

Surowiec, Aa.; Pomorski, K.; Schmitt, Ch.; Bartel, J.

2002-01-01

The emission widths Γ n and Γ p for emission of neutrons and protons are calculated within the Thomas-Fermi model, which we have recently developed, and are compared with those obtained in the usual Weisskopf approach for the case of zero angular momentum. Both methods yield quite similar results at small deformations, but rather important differences are observed for very deformed shapes, in particular for charged particles. A possible generalization of the model for emission of α-particles is also discussed. (author)

Fast Flows in the Magnetotail and Energetic Particle Transport: Multiscale Coupling in the Magnetosphere

Science.gov (United States)

Lin, Y.; Wang, X.; Fok, M. C. H.; Buzulukova, N.; Perez, J. D.; Chen, L. J.

2017-12-01

The interaction between the Earth's inner and outer magnetospheric regions associated with the tail fast flows is calculated by coupling the Auburn 3-D global hybrid simulation code (ANGIE3D) to the Comprehensive Inner Magnetosphere/Ionosphere (CIMI) model. The global hybrid code solves fully kinetic equations governing the ions and a fluid model for electrons in the self-consistent electromagnetic field of the dayside and night side outer magnetosphere. In the integrated computation model, the hybrid simulation provides the CIMI model with field data in the CIMI 3-D domain and particle data at its boundary, and the transport in the inner magnetosphere is calculated by the CIMI model. By joining the two existing codes, effects of the solar wind on particle transport through the outer magnetosphere into the inner magnetosphere are investigated. Our simulation shows that fast flows and flux ropes are localized transients in the magnetotail plasma sheet and their overall structures have a dawn-dusk asymmetry. Strong perpendicular ion heating is found at the fast flow braking, which affects the earthward transport of entropy-depleted bubbles. We report on the impacts from the temperature anisotropy and non-Maxwellian ion distributions associated with the fast flows on the ring current and the convection electric field.

Particle and VOC emission factor measurements for anthropogenic sources in West Africa

Directory of Open Access Journals (Sweden)

S. Keita

2018-06-01

Full Text Available A number of campaigns have been carried out to establish the emission factors of pollutants from fuel combustion in West Africa, as part of work package 2 (Air Pollution and Health of the DACCIWA (Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa FP7 program. Emission sources considered here include wood (hevea and iroko and charcoal burning, charcoal making, open trash burning, and vehicle emissions, including trucks, cars, buses and two-wheeled vehicles. Emission factors of total particulate matter (TPM, elemental carbon (EC, primary organic carbon (OC and volatile organic compounds (VOCs have been established. In addition, emission factor measurements were performed in combustion chambers in order to reproduce field burning conditions for a tropical hardwood (hevea, and obtain particulate emission factors by size (PM0.25, PM1, PM2.5 and PM10. Particle samples were collected on quartz fiber filters and analyzed using gravimetric method for TPM and thermal methods for EC and OC. The emission factors of 58 VOC species were determined using offline sampling on a sorbent tube. Emission factor results for two species of tropical hardwood burning of EC, OC and TPM are 0.98 ± 0.46 g kg−1 of fuel burned (g kg−1, 11.05 ± 4.55 and 41.12 ± 24.62 g kg−1, respectively. For traffic sources, the highest emission factors among particulate species are found for the two-wheeled vehicles with two-stroke engines (2.74 g kg−1 fuel for EC, 65.11 g kg−1 fuel for OC and 496 g kg−1 fuel for TPM. The largest VOC emissions are observed for two-stroke two-wheeled vehicles, which are up to 3 times higher than emissions from light-duty and heavy-duty vehicles. Isoprene and monoterpenes, which are usually associated with biogenic emissions, are present in almost all anthropogenic sources investigated during this work and could be as significant as aromatic emissions in wood burning (1 g kg−1 fuel. EC is

African Anthropogenic Emissions Inventories for gases and particles from 1990 to 2016

Science.gov (United States)

Liousse, Catherine; Keita, Sekou; N'Datchoch Touré, Evelyne 1; Doumbia, Thierno; Yoboué, Véronique; Assamoi, Eric; Haslett, Sophie; Roblou, Laurent; Léon, Jean-François; Galy-Lacaux, Corinne; Akpo, Aristide; Coe, Hugh

2017-04-01

Presently, there is one African regional inventory dealing with biofuel and fossil fuel emissions (Liousse et al., 2014) and only global emission inventories including Africa. Developing a regional inventory for gases and particles is not an easy task: the DACCIWA project has allowed to organize a framework suitable for this development through regrouping several investigators. The aim is to set an African database on fuel consumption and new emission factor measurements and to include other sources of pollution than biofuel and fossil fuel such as flaring and waste burning yet not negligible in Africa. The inclusion of these sources in the new inventory and also new emissions factor measurements will reduce the uncertainties on anthropogenic emissions in Africa. This work will present the first version of African fossil fuel (FF), biofuel (BF), gas flaring and waste burning emission inventories for the 1990-2016 period for the major atmospheric compounds (gases and particles) provides up to date emission fields at 0.125° x 0.125° spatial resolution and yearly temporal resolution that can be used to model atmospheric composition and impacts over West Africa. New emission factor measurements on ground and in combustion chambers will be discussed. Temporal variability of emissions from 1990 to 2016 will be scrutinized. In parallel, uncertainties on existing biomass burning emission inventories will be presented. New emission inventories based on MODIS burnt area products and AMMABB methodology have been developed for the period 2000-2012. They will be compared with GFED and GFAS products. Finally, tests on these inventories in Regional Climate Model (RegCM) at African scale will be presented for different years.

Timescale of particle emission using nuclear interferometry

International Nuclear Information System (INIS)

Ardouin, D.; Goujdami, D.; Guilbault, F.; Lebrun, C.; Erazmus, B.; Dabrowski, H.; Durand, D.; Lautridou, P.; Boisgard, R.; Quebert, J.; Carjan, N.

1989-01-01

A review of meson and baryon correlations at various energies is presented. An attempt, to focus on possible lifetime effects contained in existing data,is made. Data at 94 and 44 MeV/u, where experimental conditions are chosen, trying to study the lifetime of light particle emission using two particle correlations, are discussed. The temperature of a thermalized system is obtained, using the relative population of cluster excited states. It is shown that either quantum statistical fluctuations or Coulomb interactions play an important role in the trends of the correlation-functions at very low relative momenta. In the case of 1 60 and Ar induced reactions on heavy targets, a lifetime of the order of 10 -21 seconds is estimated. Temperature measurements for Ar + Ag system show that part of the excitation energy is not converted into thermal energy

Innershell ionization by fast protons, alpha particles and carbon ions

International Nuclear Information System (INIS)

Dijk, J.H. van.

1984-01-01

The subject of this thesis is the study of inner-shell excitations of atoms induced by fast charged particle collisions. A new method is described for measuring the spectrum of delta-electrons emitted by 208 Pb after excitation by 15 MeV protons or 50 MeV alpha particles. Experimental equipment is described. Results of both experiments are presented and compared with PWBA models and with calculations based on a semi-classical approximation. The small-impact-parameter ionization probabilities obtained are then compared with literature. Also small-impact-parameter measurements done with 100 MeV carbon ions are described. Besides K-shell measurements, the author also presents L-subshell ionization probability results for Pb. An appendix is added in which energy straggling problems in solid targets are treated. (Auth./G.J.P.)

Emissions and measure analysis of fine particles 2000-2020; Emissionen und Massnahmenanalyse Feinstaub 2000-2020

Energy Technology Data Exchange (ETDEWEB)

Joerss, Wolfram; Handke, Volker [Institut fuer Zukunftsstudien und Technologiebewertung gGmbH (IZT), Berlin (Germany)

2007-08-15

With this study, the Federal Environmental Agency's emission inventory on total suspended particles and the fine fractions PM{sub 1}0 and PM{sub 2}.5 was updated. On that basis, a reference scenario was developed for anthropogenic emissions of particulate matter up to the years 2010, 2015 and 2020. In addition, potential additional emission reduction measures were systematically collected and quantified. At the source groups which contribute most strongly to the emissions there are clear differences between the fine fractions and in the course of time. In particular, with the total fine the emission freight is very broadly distributed over many source groups. With PM{sub 2}.5, the emissions are more strongly concentrated on a limited number of source groups. The decrease of the emissions in the years between 2000 and 2020 in the reference scenario takes place in source groups with high portions of PM{sub 2}.5 of the emissions of total fine particles.

Emissions and measure analysis of fine particles 2000-2020; Emissionen und Massnahmenanalyse Feinstaub 2000-2020

Energy Technology Data Exchange (ETDEWEB)

Joerss, Wolfram; Handke, Volker [Institut fuer Zukunftsstudien und Technologiebewertung gGmbH (IZT), Berlin (Germany)

2007-08-15

With this study, the Federal Environmental Agency's emission inventory on total suspended particles and the fine fractions PM{sub 1}0 and PM{sub 2}.5 was updated. On that basis, a reference scenario was developed for anthropogenic emissions of particulate matter up to the years 2010, 2015 and 2020. In addition, potential additional emission reduction measures were systematically collected and quantified. At the source groups which contribute most strongly to the emissions there are clear differences between the fine fractions and in the course of time. In particular, with the total fine the emission freight is very broadly distributed over many source groups. With PM{sub 2}.5, the emissions are more strongly concentrated on a limited number of source groups. The decrease of the emissions in the years between 2000 and 2020 in the reference scenario takes place in source groups with high portions of PM{sub 2}.5 of the emissions of total fine particles.

Description of light charged particle emission in ternary fission

International Nuclear Information System (INIS)

Andreev, A. V.; Adamian, G. G.; Antonenko, N. V.; Kuklin, S. N.; Scheid, W.

2010-01-01

We consider the motion of three fragments starting from the scission point of ternary system. In the alpha-accompanied ternary fission the initial conditions are not the free parameters and determined by minimization of potential energy at scission point. In the trajectory calculations the angular distribution and mean value of the kinetic energy of the alpha-particles are well described in the spontaneous ternary fission of 252 Cf. In the Be- and C-accompanied ternary fission we found that the emission of the third particle occurs from one of the heavy fragments after their separation. (authors)

Particle and carbon dioxide emissions from passenger vehicles operating on unleaded petrol and LPG fuel

International Nuclear Information System (INIS)

Ristovski, Z.D.; Jayaratne, E.R.; Morawska, L.; Ayoko, G.A.; Lim, M.

2005-01-01

A comprehensive study of the particle and carbon dioxide emissions from a fleet of six dedicated liquefied petroleum gas (LPG) powered and five unleaded petrol (ULP) powered new Ford Falcon Forte passenger vehicles was carried out on a chassis dynamometer at four different vehicle speeds-0 (idle), 40, 60, 80 and 100 km h -1 . Emission factors and their relative values between the two fuel types together with a statistical significance for any difference were estimated for each parameter. In general, LPG was found to be a 'cleaner' fuel, although in most cases, the differences were not statistically significant owing to the large variations between emissions from different vehicles. The particle number emission factors ranged from 10 11 to 10 13 km -1 and was over 70% less with LPG compared to ULP. Corresponding differences in particle mass emission factor between the two fuels were small and ranged from the order of 10 μg km -1 at 40 to about 1000 μg km -1 at 100 km h -1 . The count median particle diameter (CMD) ranged from 20 to 35 nm and was larger with LPG than with ULP in all modes except the idle mode. Carbon dioxide emission factors ranged from about 300 to 400 g km -1 at 40 km h -1 , falling with increasing speed to about 200 g km -1 at 100 km h -1 . At all speeds, the values were 10% to 18% greater with ULP than with LPG

Electrochemical etching amplification of low-let recoil particle tracks in polymers for fast neutron dosimetry

International Nuclear Information System (INIS)

Sohrabi, M.; Morgan, K.Z.

1975-11-01

An electrochemical etching method for the amplification of fast-neutron-induced recoil particle tracks in polymers was investigated. The technique gave superior results over those obtained by conventional etching methods especially when polycarbonate foils were used for recoil particle track amplification. Electrochemical etching systems capable of multi-foil processing were designed and constructed to demonstrate the feasibility of the techniques for large-scale neutron dosimetry. Electrochemical etching parameters were studied including the nature or type of the polymer foil used, foil thickness and its effect on etching time, the applied voltage and its frequency, the chemical composition, concentration, and temperature of the etchant, distance and angle between the electrodes, and the type of particles such as recoil particles including protons. Recoil particle track density, mean track diameter, and optical density as functions of the mentioned parameters were determined. Each parameter was found to have a distinct effect on the etching results in terms of the measured responses. Several new characteristics of this fast neutron dosimetry method were studied especially for personnel dosimetry using various radiation sources such as nuclear reactors, medical cyclotrons, and isotopic neutron sources. The dose range, neutron energy dependence, directional response, fading characteristics, neutron threshold energy, etc. were investigated

Emission of complex particles from highly excited nuclei

International Nuclear Information System (INIS)

Gadioli, E.

1984-01-01

A great deal of work has been made to investigated experimentally and predict theoretically the continuous spectra of composite particles produced in reactions induced by nucleons with energy ranging from a few to several ten MeV. Some recent results in the field are summarized. In particular the exciton coalescence-pickup model and the exciton knock-on model, in the case of alpha emission, are reviewed and discussed

Diesel passenger car PM emissions: From Euro 1 to Euro 4 with particle filter

Science.gov (United States)

Tzamkiozis, Theodoros; Ntziachristos, Leonidas; Samaras, Zissis

2010-03-01

This paper examines the impact of the emission control and fuel technology development on the emissions of gaseous and, in particular, PM pollutants from diesel passenger cars. Three cars in five configurations in total were measured, and covered the range from Euro 1 to Euro 4 standards. The emission control ranged from no aftertreatment in the Euro 1 case, an oxidation catalyst in Euro 2, two oxidation catalysts and exhaust gas recirculation in Euro 3 and Euro 4, while a catalyzed diesel particle filter (DPF) fitted in the Euro 4 car led to a Euro 4 + DPF configuration. Both certification test and real-world driving cycles were employed. The results showed that CO and HC emissions were much lower than the emission standard over the hot-start real-world cycles. However, vehicle technologies from Euro 2 to Euro 4 exceeded the NOx and PM emission levels over at least one real-world cycle. The NOx emission level reached up to 3.6 times the certification level in case of the Euro 4 car. PM were up to 40% and 60% higher than certification level for the Euro 2 and Euro 3 cars, while the Euro 4 car emitted close or slightly below the certification level over the real-world driving cycles. PM mass reductions from Euro 1 to Euro 4 were associated with a relevant decrease in the total particle number, in particular over the certification test. This was not followed by a respective reduction in the solid particle number which remained rather constant between the four technologies at 0.86 × 10 14 km -1 (coefficient of variation 9%). As a result, the ratio of solid vs. total particle number ranged from ˜50% in Euro 1-100% in Euro 4. A significant reduction of more than three orders of magnitude in solid particle number is achieved with the introduction of the DPF. However, the potential for nucleation mode formation at high speed from the DPF car is an issue that needs to be considered in the over all assessment of its environmental benefit. Finally, comparison of the

Size-selective sorting in bubble streaming flows: Particle migration on fast time scales

Science.gov (United States)

Thameem, Raqeeb; Rallabandi, Bhargav; Hilgenfeldt, Sascha

2015-11-01

Steady streaming from ultrasonically driven microbubbles is an increasingly popular technique in microfluidics because such devices are easily manufactured and generate powerful and highly controllable flows. Combining streaming and Poiseuille transport flows allows for passive size-sensitive sorting at particle sizes and selectivities much smaller than the bubble radius. The crucial particle deflection and separation takes place over very small times (milliseconds) and length scales (20-30 microns) and can be rationalized using a simplified geometric mechanism. A quantitative theoretical description is achieved through the application of recent results on three-dimensional streaming flow field contributions. To develop a more fundamental understanding of the particle dynamics, we use high-speed photography of trajectories in polydisperse particle suspensions, recording the particle motion on the time scale of the bubble oscillation. Our data reveal the dependence of particle displacement on driving phase, particle size, oscillatory flow speed, and streaming speed. With this information, the effective repulsive force exerted by the bubble on the particle can be quantified, showing for the first time how fast, selective particle migration is effected in a streaming flow. We acknowledge support by the National Science Foundation under grant number CBET-1236141.

Particle number and particulate mass emissions of heavy duty vehicles in real operating conditions

Directory of Open Access Journals (Sweden)

Rymaniak Lukasz

2017-01-01

Full Text Available The article investigates the issue of PM emissions from HDV vehicles. The theoretical part discusses the problem of emission of this toxic compound in terms of particle structure taking into account the mass and dimensions of PM. Next, the methodology of the research and the results of the measurements performed under the conditions of actual operation were presented. The test drive routes were chosen in accordance with the operational purpose of the selected test vehicles. Two heavy vehicles were used for the study: a tractor with trailer and an eighteen meter long city bus. The test vehicles complied with the Euro V standard, with the second vehicle additionally complying with the EEV standard and being equipped with a DPF. The analysis of the research results was performed in the aspect of determining the operating time densities of vehicles and their drive systems as well as defining their emission characteristics and ecological indicators. PM and PN emissions were measured in the tests and particle size distribution was determined. It was shown that the exhaust gas after treatment system used in the city bus had a positive influence on the ecological indicators and had contributed to the reduction of PN emissions for heavier particles.

Fission-neutrons source with fast neutron-emission timing

Energy Technology Data Exchange (ETDEWEB)

Rusev, G., E-mail: rusev@lanl.gov; Baramsai, B.; Bond, E.M.; Jandel, M.

2016-05-01

A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of {sup 252}Cf. The time is provided by registering the fission fragments in a layer of a thin scintillation film with a signal rise time of 1 ns. The scintillation light output is measured by two silicon photomultipliers with rise time of 0.5 ns. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements using it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.

Airborne particle emission of a commercial 3D printer: the effect of filament material and printing temperature.

Science.gov (United States)

Stabile, L; Scungio, M; Buonanno, G; Arpino, F; Ficco, G

2017-03-01

The knowledge of exposure to the airborne particle emitted from three-dimensional (3D) printing activities is becoming a crucial issue due to the relevant spreading of such devices in recent years. To this end, a low-cost desktop 3D printer based on fused deposition modeling (FDM) principle was used. Particle number, alveolar-deposited surface area, and mass concentrations were measured continuously during printing processes to evaluate particle emission rates (ERs) and factors. Particle number distribution measurements were also performed to characterize the size of the emitted particles. Ten different materials and different extrusion temperatures were considered in the survey. Results showed that all the investigated materials emit particles in the ultrafine range (with a mode in the 10-30-nm range), whereas no emission of super-micron particles was detected for all the materials under investigation. The emission was affected strongly by the extrusion temperature. In fact, the ERs increase as the extrusion temperature increases. Emission rates up to 1×10 12  particles min -1 were calculated. Such high ERs were estimated to cause large alveolar surface area dose in workers when 3D activities run. In fact, a 40-min-long 3D printing was found to cause doses up to 200 mm 2 . © 2016 John Wiley & Sons A/S. Published by John Wiley & Sons Ltd.

Influence of firebed temperature on inorganic particle emissions in a residential wood pellet boiler

Science.gov (United States)

Gehrig, Matthias; Jaeger, Dirk; Pelz, Stefan K.; Weissinger, Alexander; Groll, Andreas; Thorwarth, Harald; Haslinger, Walter

2016-07-01

The temperature-dependent release of inorganic elements is the first step of the main formation pathway of particle emissions in automatically fired biomass burners. To investigate this step, a residential pellet boiler with an underfeed-burner was equipped with a direct firebed cooling. This test setup enabled decreased firebed temperatures without affecting further parameters like air flow rates or oxygen content in the firebed. A reduction of particle emissions in PM1-fraction at activated firebed cooling was found by impactor measurement and by optical particle counter. The affected particles were found in the size range boiler ash showed no statistically significant differences due to the firebed cooling. Therefore, our results indicate that the direct firebed cooling influenced the release of potassium (K) without affecting other chemical reactions.

Effects of fresh lubricant oils on particle emissions emitted by a modern gasoline direct injection passenger car.

Science.gov (United States)

Pirjola, Liisa; Karjalainen, Panu; Heikkilä, Juha; Saari, Sampo; Tzamkiozis, Theodoros; Ntziachristos, Leonidas; Kulmala, Kari; Keskinen, Jorma; Rönkkö, Topi

2015-03-17

Particle emissions from a modern turbocharged gasoline direct injection passenger car equipped with a three-way catalyst and an exhaust gas recirculation system were studied while the vehicle was running on low-sulfur gasoline and, consecutively, with five different lubrication oils. Exhaust particle number concentration, size distribution, and volatility were determined both at laboratory and on-road conditions. The results indicated that the choice of lubricant affected particle emissions both during the cold start and warm driving cycles. However, the contribution of engine oil depended on driving conditions being higher during acceleration and steady state driving than during deceleration. The highest emission factors were found with two oils that had the highest metal content. The results indicate that a 10% decrease in the Zn content of engine oils is linked with an 11-13% decrease to the nonvolatile particle number emissions in steady driving conditions and a 5% decrease over the New European Driving Cycle. The effect of lubricant on volatile particles was even higher, on the order of 20%.

Electron Cyclotron Maser Emissions from Evolving Fast Electron Beams

Science.gov (United States)

Tang, J. F.; Wu, D. J.; Chen, L.; Zhao, G. Q.; Tan, C. M.

2016-05-01

Fast electron beams (FEBs) are common products of solar active phenomena. Solar radio bursts are an important diagnostic tool for understanding FEBs and the solar plasma environment in which they propagate along solar magnetic fields. In particular, the evolution of the energy spectrum and velocity distribution of FEBs due to the interaction with the ambient plasma and field during propagation can significantly influence the efficiency and properties of their emissions. In this paper, we discuss the possible evolution of the energy spectrum and velocity distribution of FEBs due to energy loss processes and the pitch-angle effect caused by magnetic field inhomogeneity, and we analyze the effects of the evolution on electron-cyclotron maser (ECM) emission, which is one of the most important mechanisms for producing solar radio bursts by FEBs. Our results show that the growth rates all decrease with the energy loss factor Q, but increase with the magnetic mirror ratio σ as well as with the steepness index δ. Moreover, the evolution of FEBs can also significantly influence the fastest growing mode and the fastest growing phase angle. This leads to the change of the polarization sense of the ECM emission. In particular, our results also reveal that an FEB that undergoes different evolution processes will generate different types of ECM emission. We believe the present results to be very helpful for a more comprehensive understanding of the dynamic spectra of solar radio bursts.

ELECTRON CYCLOTRON MASER EMISSIONS FROM EVOLVING FAST ELECTRON BEAMS

International Nuclear Information System (INIS)

Tang, J. F.; Wu, D. J.; Chen, L.; Zhao, G. Q.; Tan, C. M.

2016-01-01

Fast electron beams (FEBs) are common products of solar active phenomena. Solar radio bursts are an important diagnostic tool for understanding FEBs and the solar plasma environment in which they propagate along solar magnetic fields. In particular, the evolution of the energy spectrum and velocity distribution of FEBs due to the interaction with the ambient plasma and field during propagation can significantly influence the efficiency and properties of their emissions. In this paper, we discuss the possible evolution of the energy spectrum and velocity distribution of FEBs due to energy loss processes and the pitch-angle effect caused by magnetic field inhomogeneity, and we analyze the effects of the evolution on electron-cyclotron maser (ECM) emission, which is one of the most important mechanisms for producing solar radio bursts by FEBs. Our results show that the growth rates all decrease with the energy loss factor Q , but increase with the magnetic mirror ratio σ as well as with the steepness index δ . Moreover, the evolution of FEBs can also significantly influence the fastest growing mode and the fastest growing phase angle. This leads to the change of the polarization sense of the ECM emission. In particular, our results also reveal that an FEB that undergoes different evolution processes will generate different types of ECM emission. We believe the present results to be very helpful for a more comprehensive understanding of the dynamic spectra of solar radio bursts.

Ethanol emission from loose corn silage and exposed silage particles

Science.gov (United States)

Hafner, Sasha D.; Montes, Felipe; Rotz, C. Alan; Mitloehner, Frank

2010-11-01

Silage on dairy farms has been identified as a major source of volatile organic compound (VOC) emissions. However, rates of VOC emission from silage are not accurately known. In this work, we measured ethanol (a dominant silage VOC) emission from loose corn silage and exposed corn silage particles using wind tunnel systems. Flux of ethanol was highest immediately after exposing loose silage samples to moving air (as high as 220 g m -2 h -1) and declined by as much as 76-fold over 12 h as ethanol was depleted from samples. Emission rate and cumulative 12 h emission increased with temperature, silage permeability, exposed surface area, and air velocity over silage samples. These responses suggest that VOC emission from silage on farms is sensitive to climate and management practices. Ethanol emission rates from loose silage were generally higher than previous estimates of total VOC emission rates from silage and mixed feed. For 15 cm deep loose samples, mean cumulative emission was as high as 170 g m -2 (80% of initial ethanol mass) after 12 h of exposure to an air velocity of 5 m s -1. Emission rates measured with an emission isolation flux chamber were lower than rates measured in a wind tunnel and in an open setting. Results show that the US EPA emission isolation flux chamber method is not appropriate for estimating VOC emission rates from silage in the field.

Evaluation of methods for the physical characterization of the fine particle emissions from two residential wood combustion appliances

Science.gov (United States)

Kinsey, John S.; Kariher, Peter H.; Dong, Yuanji

The fine particle emissions from a U. S. certified non-catalytic wood stove and a zero-clearance fireplace burning Quercus rubra L. (northern red oak) and Pseudotsuga menziesii (Douglas fir) cordwood each at two different moisture levels were determined. Emission testing was performed using both time-integrated and continuous instrumentation for total particle mass, particle number, particle size distribution, and fixed combustion gases using an atmospheric wind tunnel, full-flow laboratory dilution tunnel, and dilution stack sampler with a comparison made between the three dilution systems and two sampling filter types. The total mass emission factors (EFs) for all dilution systems and filter media are extremely variable ranging from fireplace emissions burning wet oak averaged 11 g kg -1. A substantial number of ultrafine particles in the accumulation size range were also observed during all tests as determined by an Electrical Low Pressure Impactor (ELPI) and Scanning Mobility Particle Sizer. The PM-2.5 (particles ≤2.5 μm in aerodynamic diameter) fractions determined from the ELPI electrometer data ranged from 93 to 98% (mass) depending on appliance type as reported previously by Hays et al. (Aerosol Science, 34, 1061, 2003).

Climate effects of a hypothetical regional nuclear war: Sensitivity to emission duration and particle composition

Science.gov (United States)

Pausata, Francesco S. R.; Lindvall, Jenny; Ekman, Annica M. L.; Svensson, Gunilla

2016-11-01

Here, we use a coupled atmospheric-ocean-aerosol model to investigate the plume development and climate effects of the smoke generated by fires following a regional nuclear war between emerging third-world nuclear powers. We simulate a standard scenario where 5 Tg of black carbon (BC) is emitted over 1 day in the upper troposphere-lower stratosphere. However, it is likely that the emissions from the fires ignited by bomb detonations include a substantial amount of particulate organic matter (POM) and that they last more than 1 day. We therefore test the sensitivity of the aerosol plume and climate system to the BC/POM ratio (1:3, 1:9) and to the emission length (1 day, 1 week, 1 month). We find that in general, an emission length of 1 month substantially reduces the cooling compared to the 1-day case, whereas taking into account POM emissions notably increases the cooling and the reduction of precipitation associated with the nuclear war during the first year following the detonation. Accounting for POM emissions increases the particle size in the short-emission-length scenarios (1 day/1 week), reducing the residence time of the injected particle. While the initial cooling is more intense when including POM emission, the long-lasting effects, while still large, may be less extreme compared to the BC-only case. Our study highlights that the emission altitude reached by the plume is sensitive to both the particle type emitted by the fires and the emission duration. Consequently, the climate effects of a nuclear war are strongly dependent on these parameters.

Alpha-particle emission probabilities in the decay of 239Pu

International Nuclear Information System (INIS)

Garcia-Torano, E.; Acena, M.L.; Bortels, G.; Mouchel, D.

1993-01-01

The alpha-particle emission probabilities (P α ) of 239 Pu have been measured using material of highest enrichment and radiochemical purity, thin sources produced by vacuum sublimation, and high-resolution α spectroscopy with ion-implanted Si detectors (PIPS). The results for the major emissions are P α0.07 =0.7077±0.0014, P α13 =0.1711±0.0014 and P α51 =0.1194±0.0007, which for the P α0.07 is about 3.6% lower than the recent evaluated value in the literature. (orig.)

Estimation of the time scale of last chance alpha emission using an ''atomic clock''

International Nuclear Information System (INIS)

Gallamore, L.; Sarantites, D.G.; Charity, R.J.; Nicolis, N.G.; Sobotka, L.G.; Beene, J.R.; Halbert, M.L.; Varner, R.L.

1994-01-01

The probability of filling a K-vacancy, created on the incoming part of the collision, before α-particle emission is used to time the decay of Yb compound nuclei. These nuclei were produced in the fusion reaction 250 MeV 60 Ni+ 100 Mo. In general the nuclear decays are too fast to be timed by this clock, however, α-particle emitting compound nucleus states have lifetimes sufficiently long for this technique to work when both the α-particle has low energy and the compound nucleus spin is large. This supports the existence of last, or near last, chance α-particle emission in the deexcitation of high spin compound nuclei

On the acceleration of alpha particles in the fast solar wind

International Nuclear Information System (INIS)

Gomberoff, L.; Hernandez, R.

1992-01-01

Recently, Gomberoff and Elgueta (1991) showed that in a plasma composed of anisotropic protons and alpha particles drifting along an external magnetic field with a small velocity relative to the protons, strong left-hand polarized electromagnetic ion cyclotron waves can be generated. These waves can accelerate the alpha particles to velocities well in excess of the proton bulk velocity. Here the authors assume a more realistic model of the solar wind by considering a double-humped proton distribution. It is shown that the secondary proton beam has no important effects on the ion cyclotron waves for beam densities of the order of those observed in fast solar wind conditions. The fact that the alpha proton drift velocity is modulated by the Alfven velocity remains unexplained

Particle and NO{sub x} Emissions from a HVO-Fueled Diesel Engine

Energy Technology Data Exchange (ETDEWEB)

Happonen, M.

2012-10-15

Concerns about oil price, the strengthening climate change and traffic related health effects are all reasons which have promoted the research of renewable fuels. One renewable fuel candidate is diesel consisting of hydrotreated vegetable oils (HVO). The fuel is essentially paraffinic, has high cetane number (>80) and contains practically no oxygen, aromatics or sulphur. Furthermore, HVO fuel can be produced from various feedstocks including palm, soybean and rapeseed oils as well as animal fats. HVO has also been observed to reduce all regulated engine exhaust emissions compared to conventional diesel fuel. In this thesis, the effect of HVO fuel on engine exhaust emissions has been studied further. The thesis is roughly divided into two parts. The first part explores the emission reductions associated with the fuel and studies techniques which could be applied to achieve further emission reductions. One of the studied techniques was adjusting engine settings to better suit HVO fuel. The settings chosen for adjustments were injection pressure, injection timing, the amount of EGR and the timing of inlet valve closing (with constant inlet air mass flow, i.e. Miller timing). The engine adjustments were also successfully targeted to reduce either NO{sub x} or particulate emissions or both. The other applied emission reduction technique was the addition of oxygenate to HVO fuel. The chosen oxygenate was di-n-pentyl ether (DNPE), and tested fuel blend included 20 wt-% DNPE and 80 wt-% HVO. Thus, the oxygen content of the resulting blend was 2 wt-%. Reductions of over 25 % were observed in particulate emissions with the blend compared to pure HVO while NOx emissions altered under 5 %. On the second part of this thesis, the effect of the studied fuels on chosen surface properties of exhaust particles were studied using tandem differential mobility analyzer (TDMA) techniques and transmission electron microscopy (TEM). The studied surface properties were oxidizability and

Electromagnetic scattering and emission by a fixed multi-particle object in local thermal equilibrium: General formalism.

Science.gov (United States)

Mishchenko, Michael I

2017-10-01

The majority of previous studies of the interaction of individual particles and multi-particle groups with electromagnetic field have focused on either elastic scattering in the presence of an external field or self-emission of electromagnetic radiation. In this paper we apply semi-classical fluctuational electrodynamics to address the ubiquitous scenario wherein a fixed particle or a fixed multi-particle group is exposed to an external quasi-polychromatic electromagnetic field as well as thermally emits its own electromagnetic radiation. We summarize the main relevant axioms of fluctuational electrodynamics, formulate in maximally rigorous mathematical terms the general scattering-emission problem for a fixed object, and derive such fundamental corollaries as the scattering-emission volume integral equation, the Lippmann-Schwinger equation for the dyadic transition operator, the multi-particle scattering-emission equations, and the far-field limit. We show that in the framework of fluctuational electrodynamics, the computation of the self-emitted component of the total field is completely separated from that of the elastically scattered field. The same is true of the computation of the emitted and elastically scattered components of quadratic/bilinear forms in the total electromagnetic field. These results pave the way to the practical computation of relevant optical observables.

Number size distribution of fine and ultrafine fume particles from various welding processes.

Science.gov (United States)

Brand, Peter; Lenz, Klaus; Reisgen, Uwe; Kraus, Thomas

2013-04-01

Studies in the field of environmental epidemiology indicate that for the adverse effect of inhaled particles not only particle mass is crucial but also particle size is. Ultrafine particles with diameters below 100 nm are of special interest since these particles have high surface area to mass ratio and have properties which differ from those of larger particles. In this paper, particle size distributions of various welding and joining techniques were measured close to the welding process using a fast mobility particle sizer (FMPS). It turned out that welding processes with high mass emission rates (manual metal arc welding, metal active gas welding, metal inert gas welding, metal inert gas soldering, and laser welding) show mainly agglomerated particles with diameters above 100 nm and only few particles in the size range below 50 nm (10 to 15%). Welding processes with low mass emission rates (tungsten inert gas welding and resistance spot welding) emit predominantly ultrafine particles with diameters well below 100 nm. This finding can be explained by considerably faster agglomeration processes in welding processes with high mass emission rates. Although mass emission is low for tungsten inert gas welding and resistance spot welding, due to the low particle size of the fume, these processes cannot be labeled as toxicologically irrelevant and should be further investigated.

Emission temperatures from the decay of particle-unstable complex nuclei

International Nuclear Information System (INIS)

Nayak, T.K.

1990-01-01

Relative populations of particle-unstable states were measured for complex fragments emitted in the reaction 14 N + Ag at E/A = 35 MeV by using a position sensitive high resolution hodoscope. Experimental population probabilities of particle-unstable states were extracted by fitting the coincidence spectra of the decay products by an appropriate R-matrix or Breit-Wigner formalism. According to thermal models, the populations of excited states at freezeout are expected to follow a Boltzmann distribution weighted by the emission temperature of the system. Tests of this freezeout assumption were made by comparing the experimental population to the predictions of statistical calculations. Extensive statistical calculation which include the effect of sequential feeding from heavier particle unstable nuclei were performed to estimate the population probabilities and the ratios of population probabilities indicate emission temperatures of about 3-4 MeV. But a detailed comparison for individual fragments for a calculation with T em = 4 MeV reveals that about half of the measured population probabilities and one third of the ratios of the population probabilities differ significantly from the predictions of statistical calculations. Calculations which include rotational effects could not satisfactorily account for this discrepancy. These results suggest a possible breakdown of the assumption of local thermal equilibrium at freezeout

Applications of particle induced X-ray emission

International Nuclear Information System (INIS)

Akselsson, K. R.

1978-01-01

In Particle Induced X-ray Emission (PIXE) analysis samples are bombarded by protons or α-particles of a few MeV/u. The induced characteristic x-rays are detected with a x-ray detector e.g. a Si(Li)-detector. The energies of the x-ray peaks are characteristic for the elements in the samples and the intensities of the x-ray transitions are proportional to the abundances of the elements. The research area which first attracted those of us working with PIXE was the study of sources, transport and deposition of airborne particulates. Sources, transport, wet deposition, other applications where PIXE is already known to be competitive are trace elemental analysis of water below the ppb-level and analyses requiring a space resolution of 1-10μ. However, there is still much to do for physicists in developing the full potential of low-energy accelerators as analytical tools in multidisciplinary teams. (JIW)

Support vector machine to predict diesel engine performance and emission parameters fueled with nano-particles additive to diesel fuel

Science.gov (United States)

Ghanbari, M.; Najafi, G.; Ghobadian, B.; Mamat, R.; Noor, M. M.; Moosavian, A.

2015-12-01

This paper studies the use of adaptive Support Vector Machine (SVM) to predict the performance parameters and exhaust emissions of a diesel engine operating on nanodiesel blended fuels. In order to predict the engine parameters, the whole experimental data were randomly divided into training and testing data. For SVM modelling, different values for radial basis function (RBF) kernel width and penalty parameters (C) were considered and the optimum values were then found. The results demonstrate that SVM is capable of predicting the diesel engine performance and emissions. In the experimental step, Carbon nano tubes (CNT) (40, 80 and 120 ppm) and nano silver particles (40, 80 and 120 ppm) with nanostructure were prepared and added as additive to the diesel fuel. Six cylinders, four-stroke diesel engine was fuelled with these new blended fuels and operated at different engine speeds. Experimental test results indicated the fact that adding nano particles to diesel fuel, increased diesel engine power and torque output. For nano-diesel it was found that the brake specific fuel consumption (bsfc) was decreased compared to the net diesel fuel. The results proved that with increase of nano particles concentrations (from 40 ppm to 120 ppm) in diesel fuel, CO2 emission increased. CO emission in diesel fuel with nano-particles was lower significantly compared to pure diesel fuel. UHC emission with silver nano-diesel blended fuel decreased while with fuels that contains CNT nano particles increased. The trend of NOx emission was inverse compared to the UHC emission. With adding nano particles to the blended fuels, NOx increased compared to the net diesel fuel. The tests revealed that silver & CNT nano particles can be used as additive in diesel fuel to improve complete combustion of the fuel and reduce the exhaust emissions significantly.

Alpha-particle emission probabilities of ²³⁶U obtained by alpha spectrometry.

Science.gov (United States)

Marouli, M; Pommé, S; Jobbágy, V; Van Ammel, R; Paepen, J; Stroh, H; Benedik, L

2014-05-01

High-resolution alpha-particle spectrometry was performed with an ion-implanted silicon detector in vacuum on a homogeneously electrodeposited (236)U source. The source was measured at different solid angles subtended by the detector, varying between 0.8% and 2.4% of 4π sr, to assess the influence of coincidental detection of alpha-particles and conversion electrons on the measured alpha-particle emission probabilities. Additional measurements were performed using a bending magnet to eliminate conversion electrons, the results of which coincide with normal measurements extrapolated to an infinitely small solid angle. The measured alpha emission probabilities for the three main peaks - 74.20 (5)%, 25.68 (5)% and 0.123 (5)%, respectively - are consistent with literature data, but their precision has been improved by at least one order of magnitude in this work. © 2013 Published by Elsevier Ltd.

Structures in the K-shell delta electron spectrum near threshold for ionization by fast charged particles

International Nuclear Information System (INIS)

Amundsen, P.A.; Aashamar, K.

Results of calculations of the delta electron spectrum for K-shell ionization of atoms by fast charged particles for target charges in the range 6 2 <=40 are presented. Appreciable structure is found in the spectrum near the ionization threshold, in particular for fast projectiles and heavy target elements. The structure can be quite sensitive to the details of the effective atomic potentials. (Auth.)

Particles and emissions from a diesel engine equipped with a humid air motor system

Energy Technology Data Exchange (ETDEWEB)

Nord, Kent; Zurita, Grover; Tingvall, Bror; Haupt, Dan [Luleaa Univ. of Technology (Sweden). Div. of Environmental Technology

2002-02-01

A system for reduction of NO{sub x}, humid air motor system (HAM), has been connected to an eleven liters diesel engine. Earlier studies have demonstrated the system's capacity to lower NO{sub x}-emissions from diesel engines. The present study is directed to investigate their influence of the system on the emissions of particles, aldehydes and noise while at the same time monitoring essential engine parameters, water consumption and verifying the NO{sub x} reducing ability. The system has been tested under the various conditions stated in 13-mode cycle ECE R-49. Additional tests have been necessary for sampling and measurements of particles and noise. The results show that HAM caused a large reduction of the NO{sub x} emissions while the engine performance was almost unaffected. Average reduction of NO{sub x} during the different modes of ECE R-49 was 51,1%. The reduction was directly related to the humidity of the inlet air and a further reduction can be anticipated with higher humidity. Samples have also been taken for acetaldehydes and formaldehyde. The results suggest a large reduction of aldehydes, in the range of 78 to 100%, when using HAM. Unfortunately it cannot be excluded that the results obtained are a result of a combination of high air humidity and the sampling technique used. The influence of the system on the emission of hydrocarbons was negligible while a moderate increase in the emission of carbon monoxide was noticed. No confident relationship between air humidity and the observed effects could be detected. Particle number concentrations and size distribution have also been measured. The measurements showed that the particle number concentrations was usually increased when HAM was coupled to the engine. The increase in particle number concentration, observed in five out of six running modes, varied between 46 and 148%. There was no trend indicating a shift in mean particle diameter when using HAM. Noise level and cylinder pressure have also

In-situ studies on volatile jet exhaust particle emissions - impacts of fuel sulfur content and environmental conditions on nuclei-mode aerosols

Energy Technology Data Exchange (ETDEWEB)

Schroeder, F.; Baumann, R.; Petzold, A.; Busen, R.; Schulte, P.; Fiebig, M. [DLR Deutsches Zentrum fuer Luft- und Raumfahrt e.V., Wessling (Germany). Inst. fuer Physik der Atmosphaere; Brock, C.A. [Denver Univ., CO (United States). Dept. of Engineering

2000-02-01

In-situ measurements of ultrafine aerosol particle emissions were performed at cruise altitudes behind the DLR ATTAS research jet (RR M45H M501 engines) and a B737-300 aircraft (CFM56-3B1 engines). Measurements were made 0.15-20 seconds after emission as the source aircraft burned fuel with sulfur contents (FSC) of 2.6, 56 or 118 mg kg{sup -1}. Particle size distributions of from 3 to 60 nm diameter were determined using CN-counters with varying lower size detection limits. Volatile particle concentrations in the aircraft plumes strongly increased as diameter decreased toward the sizes of large molecular clusters, illustrating that apparent particle emissions are extremely sensitive to the smallest particle size detectable by the instrument used. Environmental conditions and plume age alone could influence the number of detected ultrafine (volatile) aerosols within an order of magnitude, as well. The observed volatile particle emissions decreased nonlinearly as FSC decreased to 60 mg kg{sup -1}, reaching minimum values of about 2 x 10{sup 17} kg{sup -1} and 2 x 10{sup 16} kg{sup -1} for particles >3 nm and >5 nm, respectively. Volatile particle emissions did not change significantly as FSCs were further reduced below 60 mg kg{sup -1}. Volatile particle emissions did not differ significantly between the two studied engine types. In contrast, soot particle emissions from the modern CFM56-3B1 engines were 4-5 times less (4 x 10{sup 14} kg{sup -1}) than from the older RR M45H M501 engines (1.8 x 10{sup 15} kg{sup -1}). Contrail processing has been identified as an efficient sink/quenching parameter for ultrafine particles and reduces the remaining interstitial aerosol by factors 2-10 depending on particle size.

Solid Particle Number Emission Factors of Euro VI Heavy-Duty Vehicles on the Road and in the Laboratory

Science.gov (United States)

Giechaskiel, Barouch

2018-01-01

Particulate matter (PM), and in particular ultrafine particles, have a negative impact on human health. The contribution of vehicle PM emissions to air pollution is typically quantified with emission inventories, which need vehicle emission factors as input. Heavy-duty vehicles, although they represent a small percentage of the vehicle population in nearly every major country, contribute the majority of the on-road PM emissions. However, the published data of modern heavy-duty vehicle emissions are scarce, and for the newest Euro VI technologies, almost non-existent. The main objective of this paper is to present Solid Particle Number (SPN) emission factors from Euro VI heavy-duty vehicles using diesel, Compressed Natural Gas (CNG), or Liquefied Natural Gas (LNG). Urban, rural and motorway (highway) emissions were determined on the road at various European cities using SPN Portable Emission Measurement Systems (PEMS). Additional tests on a heavy-duty chassis dynamometer showed that the solid sub-23 nm fraction, which is not covered at the moment in the European regulation, is high, especially for CNG engines. The significant contribution of regeneration events and the effect of ambient temperature and engine cold-start on particle emissions were also discussed. PMID:29425174

Solid Particle Number Emission Factors of Euro VI Heavy-Duty Vehicles on the Road and in the Laboratory

Directory of Open Access Journals (Sweden)

Barouch Giechaskiel

2018-02-01

Full Text Available Particulate matter (PM, and in particular ultrafine particles, have a negative impact on human health. The contribution of vehicle PM emissions to air pollution is typically quantified with emission inventories, which need vehicle emission factors as input. Heavy-duty vehicles, although they represent a small percentage of the vehicle population in nearly every major country, contribute the majority of the on-road PM emissions. However, the published data of modern heavy-duty vehicle emissions are scarce, and for the newest Euro VI technologies, almost non-existent. The main objective of this paper is to present Solid Particle Number (SPN emission factors from Euro VI heavy-duty vehicles using diesel, Compressed Natural Gas (CNG, or Liquefied Natural Gas (LNG. Urban, rural and motorway (highway emissions were determined on the road at various European cities using SPN Portable Emission Measurement Systems (PEMS. Additional tests on a heavy-duty chassis dynamometer showed that the solid sub-23 nm fraction, which is not covered at the moment in the European regulation, is high, especially for CNG engines. The significant contribution of regeneration events and the effect of ambient temperature and engine cold-start on particle emissions were also discussed.

Solid Particle Number Emission Factors of Euro VI Heavy-Duty Vehicles on the Road and in the Laboratory.

Science.gov (United States)

Giechaskiel, Barouch

2018-02-09

Particulate matter (PM), and in particular ultrafine particles, have a negative impact on human health. The contribution of vehicle PM emissions to air pollution is typically quantified with emission inventories, which need vehicle emission factors as input. Heavy-duty vehicles, although they represent a small percentage of the vehicle population in nearly every major country, contribute the majority of the on-road PM emissions. However, the published data of modern heavy-duty vehicle emissions are scarce, and for the newest Euro VI technologies, almost non-existent. The main objective of this paper is to present Solid Particle Number (SPN) emission factors from Euro VI heavy-duty vehicles using diesel, Compressed Natural Gas (CNG), or Liquefied Natural Gas (LNG). Urban, rural and motorway (highway) emissions were determined on the road at various European cities using SPN Portable Emission Measurement Systems (PEMS). Additional tests on a heavy-duty chassis dynamometer showed that the solid sub-23 nm fraction, which is not covered at the moment in the European regulation, is high, especially for CNG engines. The significant contribution of regeneration events and the effect of ambient temperature and engine cold-start on particle emissions were also discussed.

An experimental study of electron transfer and emission during particle-surface interactions

International Nuclear Information System (INIS)

McGrath, C.T.

2000-09-01

A new coincidence technique has been developed and used to study the secondary electron emission that arises during the interaction of ions with surfaces. This coincidence technique allows the secondary electron emission statistics due to the impact of singly, doubly and multiply charged ions on surfaces to be measured in coincidence with reflected particles, in specific charge states and with specific post-collision trajectories. This system has been used to study the impact of 8 keV H + ions on polycrystalline copper and aluminium targets. Under these conditions the potential emission contribution is negligible and the electron emission is almost entirely due to kinetic emission processes. The sub-surface contribution to the observed electron emission has been isolated using two newly developed models. These models provide valuable information about the depth and amount of surface penetration and on the probability for subsequent electron transport to the surface. The impact of 2 - 100 keV Xe q+ (q = 1 - 10) ions on polycrystalline copper has also been studied using this system. From the subsequent data the potential and kinetic contributions to secondary electron emission have been separated using a previously established model for potential emission. The resulting kinetic emission yield increases with increasing ion impact energy, consistent with current concepts on quasimolecular ionisation. For ions impacting at large incident angles evidence for sub-surface emission has also been observed. The degree of penetration increases with ion impact energy, consistent with current concepts on this effect. The formation of H - ions from incident H + ions has also been studied by measuring the secondary electron emission statistics in coincidence with reflected particles in specific final charge states. This preliminary data is consistent with a two-step process of Auger neutralisation followed by resonant electron capture to the affinity level. However this mechanism

Helium burning: a further measurement of the beta-delayed alpha-particle emission of 16 Na

International Nuclear Information System (INIS)

Gai, Moshe

1997-01-01

The 12 C (α,γ) 16 O is a key (but still unknown) reaction in helium burning. Several attempts to constrain the p-wave S-factor at Helium burning temperatures (200 M K) using the beta-delayed alpha-particle emission of 16 N have been made. However, some discrepancy exists between the spectra measured at Settle and that of TRIUMF. We have improved our previous study of the beta-delayed alpha-particle emission of 16 N by improving our statistical sample (by more than a factor of 5), improving the energy resolution of the experiment (by 20%), and in understanding our line shape, deduced from measured quantities. Our newly measured spectrum of the beta-delayed alpha-particle emission of 16 N is consistent with the Seattle ('95) data, as well as an earlier experiment performed at Mains ('71) and is not consistent with the TRIUMF ('94) data. (author)

Real-world emission factors of fine and ultrafine aerosol particles for different traffic situations in Switzerland.

Science.gov (United States)

Imhof, David; Weingartner, Ernest; Ordónez, Carlos; Gehrig, Robert; Hill, Matz; Buchmann, Brigitte; Baltensperger, Urs

2005-11-01

Extended field measurements of particle number (size distribution of particle diameters, D, in the range between 18 nm and 10 microm), surface area concentrations, and PM1 and PM10 mass concentrations were performed in Switzerland to determine traffic emissions using a comprehensive set of instruments. Measurements took place at roads with representative traffic regimes: at the kerbside of a motorway (120 km h(-1)), a highway (80-100 km h(-1)), and in an urban area with stop-and-go traffic (0-50 km h(-1)) regulated by light signals. Mean diurnal variations showed that the highest pollutant concentrations were during the morning rush hours, especially of the number density in the nanoparticle size range (D real-life" emission factors were derived using NOx concentrations to calculate dilution factors. Particle number and volume emission factors of different size ranges (18-50 nm, 18-100 nm, and 18-300 nm) were derived for the total vehicle fleet and separated into a light-duty (LDV) and a heavy-duty vehicle (HDV) contribution. The total particle number emissions per vehicle were found to be about 11.7-13.5 x 10(14) particles km(-1) for constant speed (80-120 km h(-1) and 3.9 x 10(14) particles km(-1) for urban driving conditions. LDVs showed higher emission factors at constant high speed than under urban disturbed traffic flow. In contrast, HDVs emitted more air pollutants during deceleration and acceleration processes in stop-and-go traffic than with constant speed of about 80 km h(-1). On average, one HDV emits a 10-30 times higher amount of particulate air pollutants (in terms of both number and volume) than one LDV.

Monte Carlo simulation of fast electrons and heavy particles in the CDS of nitrogen dc glow discharge

International Nuclear Information System (INIS)

Yu, W.; Zhang, L.Z.; Wang, J.L.; Han, L.; Fu, G.S.

2001-01-01

The characteristics of fast electrons (e - ) and heavy particles (N 2 + , N + , N 2f , N f ) in the cathode dark space (CDS) of nitrogen dc glow discharge are simultaneously studied by Monte Carlo simulation. The calculated energy and angular distributions of these particles at different positions from the cathode provide a clear picture of their transport behaviours within the CDS. The density and mean energy of these particles indicate that the electrons and the atomic ions (N + ) are the main high-energy species and the molecular ions (N 2 + ) are the major ions in the CDS. It can be seen from the energy distributions of the bombarding particles at the cathode surface that the molecular ions and the fast atoms (N f ) are the main active species participating in the cathode nitride material synthesis process. The influence of the backscattering of the electrons from the negative glow to the CDS is also investigated. All the calculated results provide good information on the spatial characteristics of the particles considered in this paper and also their internal connections in the CDS of nitrogen dc glow discharge. (author)

Surgical Space Suits Increase Particle and Microbiological Emission Rates in a Simulated Surgical Environment.

Science.gov (United States)

Vijaysegaran, Praveen; Knibbs, Luke D; Morawska, Lidia; Crawford, Ross W

2018-05-01

The role of space suits in the prevention of orthopedic prosthetic joint infection remains unclear. Recent evidence suggests that space suits may in fact contribute to increased infection rates, with bioaerosol emissions from space suits identified as a potential cause. This study aimed to compare the particle and microbiological emission rates (PER and MER) of space suits and standard surgical clothing. A comparison of emission rates between space suits and standard surgical clothing was performed in a simulated surgical environment during 5 separate experiments. Particle counts were analyzed with 2 separate particle counters capable of detecting particles between 0.1 and 20 μm. An Andersen impactor was used to sample bacteria, with culture counts performed at 24 and 48 hours. Four experiments consistently showed statistically significant increases in both PER and MER when space suits are used compared with standard surgical clothing. One experiment showed inconsistent results, with a trend toward increases in both PER and MER when space suits are used compared with standard surgical clothing. Space suits cause increased PER and MER compared with standard surgical clothing. This finding provides mechanistic evidence to support the increased prosthetic joint infection rates observed in clinical studies. Copyright © 2017 Elsevier Inc. All rights reserved.

Sn-doped polyhedral In2O3 particles: Synthesis, characterization, and origins of luminous emission in wide visible range

International Nuclear Information System (INIS)

Zhu Yunqing; Chen Yiqing

2012-01-01

Sn-doped octahedronal and tetrakaidecahedronal In 2 O 3 particles were successfully synthesized by simple thermal evaporation of indium grains using SnO as dopant. Structural characterization results demonstrated that the Sn-doped tetrakaidecahedronal In 2 O 3 particle had additional six {001} crystal surfaces compared with the octahedronal one. The luminous properties of both samples were characterized by photoluminescence (PL) and cathodoluminescence (CL) spectroscopy. A broad visible luminous emission around 570 nm was observed. Studies revealed that the emission consisted of three peaks of 511 nm, 564 nm, and 622 nm, which were attributed to radioactive recombination centers such as single ionized oxygen vacancy, indium interstitial, and antisite oxygen, respectively. We believe that the Sn donor level plays an important role in the visible luminous emission. - Graphical abstract: With more oxygen vacancies and tin doping. ITO particles can exhibit a better CL performance. Sn donor level near the conduction band edge plays an important role in luminous emission in wide visible range. Highlights: ► Polyhedral ITO particles synthesized by thermal evaporation using SnO as dopant. ► Broad visible luminous emission around 570 nm. ► Sn donor level plays an important role in the visible emission. ► ITO particles with more oxygen vacancies have better CL performance in visible range.

Design and construction of a fast (neutron) spectrometer for magnetic confinement fusion studies

International Nuclear Information System (INIS)

Lagattu, A.

1980-09-01

Neutron emission in conjunction with the 'Tokamak' devices studied in order to carry out controlled fusion is done at present on a short time scale (a few hundred milliseconds). Obtaining spectrometric information on this emission made it necessary to design sufficiently fast equipment to adapt to this situation. The basis of the equipment selected is conventional: NE213 liquid scintillator in conjunction with a fast photomultiplier. A commercialized fast neutron gamma discriminator (approximately 210 5 S -1 ) was used. The data acquisition and processing system was specially made for this occasion. This assembly, so designed and constructed, was tested on a particle accelerator and on the TFR Tokamak. In the best conditions a spectrum of 60 milliseconds was produced. Hence several spectra can be recorded during an experiment. The rejection of gamma radiations by the discriminator exceeds 99% in such conditions [fr

A new global particle swarm optimization for the economic emission dispatch with or without transmission losses

International Nuclear Information System (INIS)

Zou, Dexuan; Li, Steven; Li, Zongyan; Kong, Xiangyong

2017-01-01

Highlights: • A new global particle swarm optimization (NGPSO) is proposed. • NGPSO has strong convergence and desirable accuracy. • NGPSO is used to handle the economic emission dispatch with or without transmission losses. • The equality constraint can be satisfied by solving a quadratic equation. • The inequality constraints can be satisfied by using penalty function method. - Abstract: A new global particle swarm optimization (NGPSO) algorithm is proposed to solve the economic emission dispatch (EED) problems in this paper. NGPSO is different from the traditional particle swarm optimization (PSO) algorithm in two aspects. First, NGPSO uses a new position updating equation which relies on the global best particle to guide the searching activities of all particles. Second, it uses the randomization based on the uniform distribution to slightly disturb the flight trajectories of particles during the late evolutionary process. The two steps enable NGPSO to effectively execute a number of global searches, and thus they increase the chance of exploring promising solution space, and reduce the probabilities of getting trapped into local optima for all particles. On the other hand, the two objective functions of EED are normalized separately according to all candidate solutions, and then they are incorporated into one single objective function. The transformation steps are very helpful in eliminating the difference caused by the different dimensions of the two functions, and thus they strike a balance between the fuel cost and emission. In addition, a simple and common penalty function method is employed to facilitate the satisfactions of EED’s constraints. Based on these improvements in PSO, objective functions and constraints handling, high-quality solutions can be obtained for EED problems. Five examples are chosen to testify the performance of three improved PSOs on solving EED problems with or without transmission losses. Experimental results show that

Simultaneous coastal measurements of ozone deposition fluxes and iodine-mediated particle emission fluxes with subsequent CCN formation

Directory of Open Access Journals (Sweden)

J. D. Whitehead

2010-01-01

Full Text Available Here we present the first observations of simultaneous ozone deposition fluxes and ultrafine particle emission fluxes over an extensive infra-littoral zone. Fluxes were measured by the eddy covariance technique at the Station Biologique de Roscoff, on the coast of Brittany, north-west France. This site overlooks a very wide (3 km littoral zone controlled by very deep tides (9.6 m exposing extensive macroalgae beds available for significant iodine mediated photochemical production of ultrafine particles. The aspect at the Station Biologique de Roscoff provides an extensive and relatively flat, uniform fetch within which micrometeorological techniques may be utilized to study links between ozone deposition to macroalgae (and sea water and ultrafine particle production.

Ozone deposition to seawater at high tide was significantly slower (v_d[O₃]=0.302±0.095 mm s⁻¹ than low tidal deposition. A statistically significant difference in the deposition velocities to macroalgae at low tide was observed between night time (v_d[O₃]=1.00±0.10 mm s⁻¹ and daytime (v_d[O₃]=2.05±0.16 mm s⁻¹ when ultrafine particle formation results in apparent particle emission. Very high emission fluxes of ultrafine particles were observed during daytime periods at low tides ranging from 50 000 particles cm⁻² s⁻¹ to greater than 200 000 particles cm⁻² s⁻¹ during some of the lowest tides. These emission fluxes exhibited a significant relationship with particle number concentrations comparable with previous observations at another location. Apparent particle growth rates were estimated to be in the range 17–150 nm h⁻¹ for particles in the size range 3–10 nm. Under certain conditions, particle growth may be inferred to continue to greater than 120 nm over tens

Spatial distribution of {gamma} emissivity and fast ions during ({sup 3}He)D ICRF heating experiments on JET

Energy Technology Data Exchange (ETDEWEB)

Start, D F.H. [Commission of the European Communities, Abingdon (United Kingdom). JET Joint Undertaking; Righi, E [Imperial Coll. of Science and Technology, London (United Kingdom); Warrick, C [UKAEA Culham Lab., Abingdon (United Kingdom)

1994-07-01

A model is presented that can simulate the {gamma} emissivity in the poloidal cross-section during ({sup 3}He)D ICRF heated discharges in JET plasmas, by merging information obtained from the fast ion distribution and from nuclear reactions producing the observed {gamma} emissivity (production of {gamma} photons during {sup 3}He-{sup 9}Be reactions). This technique can play an important role in the identification of plasma instabilities that affect the redistribution of the fast ions in the plasma, like the TAE modes and the ripple in the tokamak magnetic field. 9 refs., 4 figs., 1 tab.

Fast emission estimates in China and South Africa constrained by satellite observations

Science.gov (United States)

Mijling, Bas; van der A, Ronald

2013-04-01

Emission inventories of air pollutants are crucial information for policy makers and form important input data for air quality models. Unfortunately, bottom-up emission inventories, compiled from large quantities of statistical data, are easily outdated for emerging economies such as China and South Africa, where rapid economic growth change emissions accordingly. Alternatively, top-down emission estimates from satellite observations of air constituents have important advantages of being spatial consistent, having high temporal resolution, and enabling emission updates shortly after the satellite data become available. However, constraining emissions from observations of concentrations is computationally challenging. Within the GlobEmission project (part of the Data User Element programme of ESA) a new algorithm has been developed, specifically designed for fast daily emission estimates of short-lived atmospheric species on a mesoscopic scale (0.25 × 0.25 degree) from satellite observations of column concentrations. The algorithm needs only one forward model run from a chemical transport model to calculate the sensitivity of concentration to emission, using trajectory analysis to account for transport away from the source. By using a Kalman filter in the inverse step, optimal use of the a priori knowledge and the newly observed data is made. We apply the algorithm for NOx emission estimates in East China and South Africa, using the CHIMERE chemical transport model together with tropospheric NO2 column retrievals of the OMI and GOME-2 satellite instruments. The observations are used to construct a monthly emission time series, which reveal important emission trends such as the emission reduction measures during the Beijing Olympic Games, and the impact and recovery from the global economic crisis. The algorithm is also able to detect emerging sources (e.g. new power plants) and improve emission information for areas where proxy data are not or badly known (e

Tomographic reconstruction by using FPSIRT (Fast Particle System Iterative Reconstruction Technique)

Energy Technology Data Exchange (ETDEWEB)

Moreira, Icaro Valgueiro M.; Melo, Silvio de Barros; Dantas, Carlos; Lima, Emerson Alexandre; Silva, Ricardo Martins; Cardoso, Halisson Alberdan C., E-mail: ivmm@cin.ufpe.br, E-mail: sbm@cin.ufpe.br, E-mail: rmas@cin.ufpe.br, E-mail: hacc@cin.ufpe.br, E-mail: ccd@ufpe.br, E-mail: eal@cin.ufpe.br [Universidade Federal de Pernambuco (UFPE), Recife, PE (Brazil)

2015-07-01

The PSIRT (Particle System Iterative Reconstruction Technique) is a method of tomographic image reconstruction primarily designed to work with configurations suitable for industrial applications. A particle system is an optimization technique inspired in real physical systems that associates to the reconstructing material a set of particles with certain physical features, subject to a force eld, which can produce movement. The system constantly updates the set of particles by repositioning them in such a way as to approach the equilibrium. The elastic potential along a trajectory is a function of the difference between the attenuation coefficient in the current configuration and the corresponding input data. PSIRT has been successfully used to reconstruct simulated and real objects subject to sets of parallel and fanbeam lines in different angles, representing typical gamma-ray tomographic arrangements. One of PSIRT's limitation was its performance, too slow for real time scenarios. In this work, it is presented a reformulation in PSIRT's computational model, which is able to grant the new algorithm, the FPSIRT - Fast System Iterative Reconstruction Technique, a performance up to 200-time faster than PSIRT's. In this work a comparison of their application to real and simulated data from the HSGT, High Speed Gamma Tomograph, is presented. (author)

Tomographic reconstruction by using FPSIRT (Fast Particle System Iterative Reconstruction Technique)

International Nuclear Information System (INIS)

Moreira, Icaro Valgueiro M.; Melo, Silvio de Barros; Dantas, Carlos; Lima, Emerson Alexandre; Silva, Ricardo Martins; Cardoso, Halisson Alberdan C.

2015-01-01

The PSIRT (Particle System Iterative Reconstruction Technique) is a method of tomographic image reconstruction primarily designed to work with configurations suitable for industrial applications. A particle system is an optimization technique inspired in real physical systems that associates to the reconstructing material a set of particles with certain physical features, subject to a force eld, which can produce movement. The system constantly updates the set of particles by repositioning them in such a way as to approach the equilibrium. The elastic potential along a trajectory is a function of the difference between the attenuation coefficient in the current configuration and the corresponding input data. PSIRT has been successfully used to reconstruct simulated and real objects subject to sets of parallel and fanbeam lines in different angles, representing typical gamma-ray tomographic arrangements. One of PSIRT's limitation was its performance, too slow for real time scenarios. In this work, it is presented a reformulation in PSIRT's computational model, which is able to grant the new algorithm, the FPSIRT - Fast System Iterative Reconstruction Technique, a performance up to 200-time faster than PSIRT's. In this work a comparison of their application to real and simulated data from the HSGT, High Speed Gamma Tomograph, is presented. (author)

Effects of a catalytic volatile particle remover (VPR) on the particulate matter emissions from a direct injection spark ignition engine.

Science.gov (United States)

Xu, Fan; Chen, Longfei; Stone, Richard

2011-10-15

Emissions of fine particles have been shown to have a large impact on the atmospheric environment and human health. Researchers have shown that gasoline engines, especially direct injection spark ignition (DISI) engines, tend to emit large amounts of small size particles compared to diesel engines fitted with diesel particulate filters (DPFs). As a result, the particle number emissions of DISI engines will be restricted by the forthcoming EU6 legislation. The particulate emission level of DISI engines means that they could face some challenges in meeting the EU6 requirement. This paper is an experimental study on the size-resolved particle number emissions from a spray guided DISI engine and the performance of a catalytic volatile particle remover (VPR), as the EU legislation seeks to exclude volatile particles. The performance of the catalytic VPR was evaluated by varying its temperature and the exhaust residence time. The effect of the catalytic VPR acting as an oxidation catalyst on particle emissions was also tested. The results show that the catalytic VPR led to a marked reduction in the number of particles, especially the smaller size (nucleation mode) particles. The catalytic VPR is essentially an oxidation catalyst, and when post three-way catalyst (TWC) exhaust was introduced to the catalytic VPR, the performance of the catalytic VPR was not affected much by the use of additional air, i.e., no significant oxidation of the PM was observed.

Characteristics of SME biodiesel-fueled diesel particle emissions and the kinetics of oxidation.

Science.gov (United States)

Jung, Heejung; Kittelson, David B; Zachariah, Michael R

2006-08-15

Biodiesel is one of the most promising alternative diesel fuels. As diesel emission regulations have become more stringent, the diesel particulate filter (DPF) has become an essential part of the aftertreatment system. Knowledge of kinetics of exhaust particle oxidation for alternative diesel fuels is useful in estimating the change in regeneration behavior of a DPF with such fuels. This study examines the characteristics of diesel particulate emissions as well as kinetics of particle oxidation using a 1996 John Deere T04045TF250 off-highway engine and 100% soy methyl ester (SME) biodiesel (B100) as fuel. Compared to standard D2 fuel, this B100 reduced particle size, number, and volume in the accumulation mode where most of the particle mass is found. At 75% load, number decreased by 38%, DGN decreased from 80 to 62 nm, and volume decreased by 82%. Part of this decrease is likely associated with the fact that the particles were more easily oxidized. Arrhenius parameters for the biodiesel fuel showed a 2-3times greater frequency factor and approximately 6 times higher oxidation rate compared to regular diesel fuel in the range of 700-825 degrees C. The faster oxidation kinetics should facilitate regeneration when used with a DPF.

Simulating emission and chemical evolution of coarse sea-salt particles in the Community Multiscale Air Quality (CMAQ) model

OpenAIRE

J. T. Kelly; P. V. Bhave; C. G. Nolte; U. Shankar; K. M. Foley

2009-01-01

Chemical processing of sea-salt particles in coastal environments significantly impacts concentrations of particle components and gas-phase species and has implications for human exposure to particulate matter and nitrogen deposition to sensitive ecosystems. Emission of sea-salt particles from the coastal surf zone is known to be elevated compared to that from the open ocean. Despite the importance of sea-salt emissions and chemical processing, the US EPA's Community Multiscale Air Quality (C...

Experimental studies on particle emissions from cruising ship, their characteristic properties, transformation and atmospheric lifetime in the marine boundary layer

Science.gov (United States)

Petzold, A.; Hasselbach, J.; Lauer, P.; Baumann, R.; Franke, K.; Gurk, C.; Schlager, H.; Weingartner, E.

2008-05-01

Particle emissions from ship engines and their atmospheric transformation in the marine boundary layer (MBL) were investigated in engine test bed studies and in airborne measurements of expanding ship plumes. During the test rig studies, detailed aerosol microphysical and chemical properties were measured in the exhaust gas of a serial MAN B&W seven-cylinder four-stroke marine diesel engine under various load conditions. The emission studies were complemented by airborne aerosol transformation studies in the plume of a large container ship in the English Channel using the DLR aircraft Falcon 20 E-5. Observations from emission studies and plume studies combined with a Gaussian plume dispersion model yield a consistent picture of particle transformation processes from emission to atmospheric processing during plume expansion. Particulate matter emission indices obtained from plume measurements are 8.8±1.0×1015(kg fuel)-1 by number for non-volatile particles and 174±43 mg (kg fuel)-1 by mass for Black Carbon (BC). Values determined for test rig conditions between 85 and 110% engine load are of similar magnitude. For the total particle number including volatile compounds no emission index can be derived since the volatile aerosol fraction is subject to rapid transformation processes in the plume. Ship exhaust particles occur in the size range Dp<0.3 μm, showing a bi-modal structure. The combustion particle mode is centred at modal diameters of 0.05 μm for raw emissions to 0.10 μm at a plume age of 1 h. The smaller-sized volatile particle mode is centred at Dp≤0.02 μm. From the decay of ship exhaust particle number concentrations in an expanding plume, a maximum plume life time of approx. 24 h is estimated for a well-mixed marine boundary layer.

Positron emission particle tracking in pulsatile flow

Energy Technology Data Exchange (ETDEWEB)

Patel, Nitant; Ruggles, Arthur [University of Tennessee-Knoxville, Department of Nuclear Engineering, Knoxville, TN (United States); Wiggins, Cody [University of Tennessee-Knoxville, Department of Physics and Astronomy, Knoxville, TN (United States)

2017-05-15

Positron emission particle tracking (PEPT) is increasingly used to understand the flow characteristics in complex systems. This research utilizes PEPT to measure pulsatile flow of frequency 2.1 Hz in an elastic Masterkleer PVC tube of 19 mm inner diameter and 3.2 mm wall thickness. Anion exchange resin beads are labeled with {sup 18}F and delivered to a pump driven flow loop with motorized ball valve used to develop the pulsatile flow. Data are collected in the tube with circular cross section, and measurements are also collected with a section of the tube pinched. Nominal flow velocities are near 1 m/s and Reynolds numbers near 20,000. Many thousand PEPT particle traces are collected and synchronized with the flow pulsation. These Lagrangian data are presented as a series of 20 still frames depicting the 3-D velocity field present during each phase of the flow pulsation. Pressure data are also collected to resolve the pressure wave front moving through the open elastic tube at velocity 15.2 m/s. (orig.)

Communications overlapping in fast multipole particle dynamics methods

International Nuclear Information System (INIS)

Kurzak, Jakub; Pettitt, B. Montgomery

2005-01-01

In molecular dynamics the fast multipole method (FMM) is an attractive alternative to Ewald summation for calculating electrostatic interactions due to the operation counts. However when applied to small particle systems and taken to many processors it has a high demand for interprocessor communication. In a distributed memory environment this demand severely limits applicability of the FMM to systems with O(10 K atoms). We present an algorithm that allows for fine grained overlap of communication and computation, while not sacrificing synchronization and determinism in the equations of motion. The method avoids contention in the communication subsystem making it feasible to use the FMM for smaller systems on larger numbers of processors. Our algorithm also facilitates application of multiple time stepping techniques within the FMM. We present scaling at a reasonably high level of accuracy compared with optimized Ewald methods

Conventional sources of fast neutrons in 'cold fusion' experiments

International Nuclear Information System (INIS)

Cribier, M.; Spiro, M.; Favier, J.

1989-04-01

In 'cold fusion' experiments with heavy water a source of neutrons is the dissociation of deuterium induced by alpha particles emitted by natural occurring radioisotopes. We evaluate the rate of fast neutron emission as a function of the concentration of U, Th, Rn in contact with deuterium and discuss the possibility that the neutrons claimed to have been observed in 'cold fusion' experiments could be due to this conventional source

The ammonium nitrate particle equivalent of NOx emissions for wintertime conditions in Central California's San Joaquin Valley

International Nuclear Information System (INIS)

Stockwell, W.R.; Watson, J.G.; Robinson, N.F.; Sylte, W.W.

2000-01-01

A new method has been developed to assess the aerosol particle formation reactivity of nitrogen oxide (NO x ) emissions. The method involves using a photochemical box model with gas-phase photochemistry, aerosol production and deposition to calculate the ammonium nitrate particle equivalent of NO x emissions. The yields of ammonium nitrate particles used in the box model were determined from parametric simulations made with an equilibrium model that calculated the fraction of nitric acid that reacts to produce ammonium nitrate from the temperature, relative humidity and ammonium-to-nitrate ratios. For the wintertime conditions of emissions and meteorology in the San Joaquin Valley of central California, approximately 80% of the moles of nitric acid produced was found to be in the particulate nitrate phase and about 33% of the moles of emitted NO x was converted to particulate nitrate. The particle equivalent of NO x emissions was found to be on the order of 0.6 g of ammonium nitrate for each gram of NO x emitted (the mass of NO x calculated as NO 2 ). This estimate is in reasonable agreement with an analysis of field measurements made in central California. (author)

Characterization of particle bound organic carbon from diesel vehicles equipped with advanced emission control technologies.

Science.gov (United States)

Pakbin, Payam; Ning, Zhi; Schauer, James J; Sioutas, Constantinos

2009-07-01

A chassis dynamometer study was carried out by the University of Southern California in collaboration with the Air Resources Board (CARB) to investigate the physical, chemical, and toxicological characteristics of diesel emissions of particulate matter (PM) from heavy-duty vehicles. These heavy-duty diesel vehicles (HDDV) were equipped with advanced emission control technologies, designed to meet CARB retrofit regulations. A HDDV without any emission control devices was used as the baseline vehicle. Three advanced emission control technologies; continuously regenerating technology (CRT), zeolite- and vanadium-based selective catalytic reduction technologies (Z-SCRT and V-SCRT), were tested under transient (UDDS) (1) and cruise (80 kmph) driving cycles to simulate real-world driving conditions. This paper focuses on the characterization of the particle bound organic species from the vehicle exhaust. Physical and chemical properties of PM emissions have been reported by Biswas et al. Atmos. Environ. 2008, 42, 5622-5634) and Hu et al. (Atmos. Environ. 2008, submitted) Significant reductions in the emission factors (microg/mile) of particle bound organic compounds were observed in HDDV equipped with advanced emission control technologies. V-SCRT and Z-SCRT effectively reduced PAHs, hopanes and steranes, n-alkanes and acids by more than 99%, and often to levels below detection limits for both cruise and UDDS cycles. The CRT technology also showed similar reductions with SCRT for medium and high molecular weight PAHs, acids, but with slightly lower removal efficiencies for other organic compounds. Ratios of particle bound organics-to-OC mass (microg/g) from the baseline exhaust were compared with their respective ratios in diesel fuel and lubricating oil, which revealed that hopanes and steranes originate from lubricating oil, whereas PAHs can either form during the combustion process or originate from diesel fuel itself. With the introduction of emission control

Aerosol and NOx emission factors and submicron particle number size distributions in two road tunnels with different traffic regimes

Directory of Open Access Journals (Sweden)

D. Imhof

2006-01-01

Full Text Available Measurements of aerosol particle number size distributions (18–700 nm, mass concentrations (PM2.5 and PM10 and NOx were performed in the Plabutsch tunnel, Austria, and in the Kingsway tunnel, United Kingdom. These two tunnels show different characteristics regarding the roadway gradient, the composition of the vehicle fleet and the traffic frequency. The submicron particle size distributions contained a soot mode in the diameter range D=80–100 nm and a nucleation mode in the range of D=20–40 nm. In the Kingsway tunnel with a significantly lower particle number and volume concentration level than in the Plabutsch tunnel, a clear diurnal variation of nucleation and soot mode particles correlated to the traffic density was observed. In the Plabutsch tunnel, soot mode particles also revealed a diurnal variation, whereas no substantial variation was found for the nucleation mode particles. During the night a higher number concentration of nucleation mode particles were measured than soot mode particles and vice versa during the day. In this tunnel with very high soot emissions during daytime due to the heavy-duty vehicle (HDV share of 18% and another 40% of diesel driven light-duty vehicles (LDV semivolatile species condense on the pre-existing soot surface area rather than forming new particles by homogeneous nucleation. With the low concentration of soot mode particles in the Kingsway tunnel, also the nucleation mode particles exhibit a diurnal variation. From the measured parameters real-world traffic emission factors were estimated for the whole vehicle fleet as well as differentiated into the two categories LDV and HDV. In the particle size range D=18–700 nm, each vehicle of the mixed fleet emits (1.50±0.08×1014 particles km-1 (Plabutsch and (1.26±0.10×1014 particles km-1 (Kingsway, while particle volume emission factors of 0.209±0.008 cm3 km-1 and 0.036±0.004 cm3 km-1, respectively, were obtained. PM1 emission factors of 104±4 mg

Emissions of air toxics from a simulated charcoal kiln. Final report, October 1997--September 1998

International Nuclear Information System (INIS)

Lemieux, P.M.

1999-06-01

The report gives results of experiments in a laboratory-scale charcoal kiln simulator to evaluate emissions of hazardous air pollutants from the production of charcoal in Missouri-type kilns. Fixed combustion gases were measured using continuous monitors. In addition, other pollutants, including methanol, volatile organic compounds, semivolatile organic compounds, and particle emission rates and size distributions were measured using various techniques. Emissions of all pollutants are reported in units of grams emitted per unit mass of initial wood converted to charcoal. Two burn conditions--slow and fast--were examined. High levels of methanol, benzene, and fine particulate were emitted in all tests. The estimated emissions from the fast burn conditions were significantly higher than those from the slow burn conditions

Ion cyclotron emission in tokamak plasmas; Emission cyclotronique ionique dans les plasmas de tokamak

Energy Technology Data Exchange (ETDEWEB)

Fraboulet, D.

1996-09-17

Detection of {alpha}(3.5 MeV) fusion products will be of major importance for the achievement of self sustained discharges in fusion thermonuclear reactors. Due to their cyclotronic gyration in the confining magnetic field of a tokamak, {alpha} particles are suspected to radiate in the radio-frequency band [RF: 10-500 MHz]. Our aim is to determine whether detection of RF emission radiated from a reactor plasma can provide information concerning those fusion products. We observed experimentally that the RF emission radiated from fast ions situated in the core of the discharge is detectable with a probe located at the plasma edge. For that purpose, fast temporal acquisition of spectral power was achieved in a narrow frequency band. We also propose two complementary models for this emission. In the first one, we describe locally the energy transfer between the photon population and the plasma and we compute the radiation equilibrium taking place in the tokamak. {alpha} particles are not the unique species involved in the equilibrium and it is necessary to take into account all other species present in the plasma (Deuterium, Tritium, electrons,...). Our second model consists in the numerical resolution of the Maxwell-Vlasov with the use of a variational formulation, in which all polarizations are considered and the 4 first cyclotronic harmonics are included in a 1-D slab geometry. The development of this second model leads to the proposal for an experimental set up aiming to the feasibility demonstration of a routine diagnostic providing the central {alpha} density in a reactor. (author). 166 refs.

Fast electrons in small solar flares

International Nuclear Information System (INIS)

Lin, R.P.

1975-01-01

Because approximately 5-100 keV electrons are frequently accelerated and emitted by the Sun in small flares, it is possible to define a detailed characteristic physical picture of these events. The review summarizes both the direct spacecraft observations of non-relativistic solar electrons, and observations of the X-ray and radio emission generated by these particles at the Sun and in the interplanetary medium. These observations bear on the basic astrophysical process of particle acceleration in tenuous plasmas. It is found that in many small solar flares the approximately 5-100 keV electrons accelerated during flash phase constitute the bulk of the total flare energy. Thus the basic flare mechanism in these flares essentially converts the available flare energy into fast electrons. These electrons may produce the other flare electromagnetic emissions through their interactions with the solar atmosphere. In large proton flares these electrons may provide the energy to eject material from the Sun and to create a shock wave which could then accelerate nuclei and electrons to much higher energies. (Auth.)

Energetic Charged Particle Emission from Hydrogen-Loaded pd and ti Cathodes and its Enhancement by He-4 Implantation

Science.gov (United States)

Lipson, A. G.; Miley, G. H.; Lipson, A. G.; Lyakhov, B. F.; Roussetski, A. S.

2006-02-01

In this paper, we demonstrate reproducible emissions of energetic alphas and protons appearing in an energy range where both cosmic ray interference and possible alpha emissions from contamination (e.g., radon) is assumed to be negligible. We also show that He4 doping of Pd and Ti cathodes leads to a significant enhancement of the energetic charged particles emission (ECPE). This measurement of the emissions of energetic (MeV) particles, in a region of low background interference plus their enhancement by He4 doping provides very strong support for the existence of LENR processes in the crystalline lattice of deuterated metals.

Energetic charged particle emission from hydrogen-loaded Pd and Ti cathodes and its enhancement by He-4 implantation

International Nuclear Information System (INIS)

Lipson, A.G.; Miley, G.H.; Lipson, A.G.; Lyakhov, B.F.; Roussetski, A.S.

2006-01-01

In this paper, we demonstrate reproducible emissions of energetic alphas and protons appearing in an energy range where both cosmic ray interference and possible alpha emissions from contamination (e.g., radon) is assumed to be negligible. We also show that, 4 He doping of Pd and Ti cathodes leads to a significant enhancement of the energetic charged particles emission (ECPE). This measurement of the emissions of energetic (MeV) particles, in a region of low background interference plus their enhancement by 4 He doping provides very strong support for the existence of LENR processes in the crystalline lattice of deuterated metals. (authors)

Investigation of p,π+- charged particle correlations in π-C interactions at 5 GeV/c with emission of a particle in the backward direction

International Nuclear Information System (INIS)

Budagov, Yu.A.; Bayaramov, A.A.; Dzhelepov, V.P.; Dvornik, A.M.; Efremov, A.V.; Flyagin, V.B.; Lomakin, Yu.F.; Valkar, S.; Volodko, A.G.

1976-01-01

The π-C interactions at 5 GeV/c are studied. Angle correlation between two charged particles when a particle is emitted to the backward hemisphere has been investigated. Noticeable correlation appears if the angle between the two particles is 180 deg (lab.s.). It follows from this behaviour that the backward emission of a particle is due to the hard collision mechanism

Determination of time- and size-dependent fine particle emission with varied oil heating in an experimental kitchen.

Science.gov (United States)

Li, Shuangde; Gao, Jiajia; He, Yiqing; Cao, Liuxu; Li, Ang; Mo, Shengpeng; Chen, Yunfa; Cao, Yaqun

2017-01-01

Particulate matter (PM) from cooking has caused seriously indoor air pollutant and aroused risk to human health. It is urged to get deep knowledge of their spatial-temporal distribution of source emission characteristics, especially ultrafine particles (UFP<100nm) and accumulation mode particles (AMP 100-665nm). Four commercial cooking oils are auto dipped water to simulate cooking fume under heating to 265°C to investigate PM emission and decay features between 0.03 and 10μm size dimension by electrical low pressure impactor (ELPI) without ventilation. Rapeseed and sunflower produced high PM 2.5 around 6.1mg/m 3 , in comparison with those of soybean and corn (5.87 and 4.65mg/m 3 , respectively) at peak emission time between 340 and 460sec since heating oil, but with the same level of particle numbers 6-9×10 5 /cm 3 . Mean values of PM 1.0 /PM 2.5 and PM 2.5 /PM 10 at peak emission time are around 0.51-0.66 and 0.23-0.29. After 15min naturally deposition, decay rates of PM 1.0 , PM 2.5 and PM 10 are 13.3%-29.8%, 20.1%-33.9% and 41.2%-54.7%, which manifest that PM 1.0 is quite hard to decay than larger particles, PM 2.5 and PM 10 . The majority of the particle emission locates at 43nm with the largest decay rate at 75%, and shifts to a larger size between 137 and 655nm after 15min decay. The decay rates of the particles are sensitive to the oil type. Copyright © 2016. Published by Elsevier B.V.

Dynamical aspects of particle emission in binary dissipative collisions -effects on hot-nuclei formation

International Nuclear Information System (INIS)

Eudes, Ph.; Basrak, Z.; Sebille, F.

1997-01-01

Characteristics of charged-particle emission in heavy-ion reactions have been studied in the framework of the semiclassical Landau-Vlasov approach for the 40 Ar + 27 Al collisions at 65 MeV/u. The reaction mechanism is dominated by binary dissipative collisions. After an abundant prompt emission coming from the overlapping region between the target and the projectile, two excited nuclei, the quasi-target and the quasi-projectile, emerge from the collision. To shed some light on the role played by dynamical effects, light-charged particle observables, which are currently used as an experimental signature a of hot equilibrated nucleus, have been carefully investigated. (K.A.)

A fast-slow logic system

International Nuclear Information System (INIS)

Kawashima, Hideo.

1977-01-01

A fast-slow logic system has been made for use in multi-detector experiments in nuclear physics such as particle-gamma and particle-particle coincidence experiments. The system consists of a fast logic system and a slow logic system. The fast logic system has a function of fast coincidences and provides timing signals for the slow logic system. The slow logic system has a function of slow coincidences and a routing control of input analog signals to the ADCs. (auth.)

The effect of fast particles' irradiation on electrooptical properties of GaP LEDs

International Nuclear Information System (INIS)

Gontaruk, O.; Kovalenko, A.; Malyj, E.; Petrenko, I.; Pinkovska, M.; Polivtcev, L.; Tartachnyk, V.

2013-01-01

The electrooptical properties of industrial AL 102 GaP light-emitting diodes (LEDs) irradiated with fast particles have been studied. 2 MeV electrons and fast reactor neutrons were used and devices' microplsma emitting, current-voltage and capacitance-voltage characteristics were measured. It was shown that electron irradiation in the range (2-5)10 16 cm -2 leads to the drop of microplasma emitting intensity, decrease of capacity and reverse currents and increase of reverse bias. The annealing study of current-voltage characteristics after neutron irradiation of diodes confirms the assumption about prevailing radiation influence on diode base due to induce of deep levels. (authors)

Size-resolved particle number emission patterns under real-world driving conditions using positive matrix factorization

NARCIS (Netherlands)

Domínguez-Sáez, A.; Viana, M.; Barrios, C.C.; Rubio, J.R.; Amato, F.; Pujadas, M.; Querol, X.

2012-01-01

A novel on-board system was tested to characterize size-resolved particle number emission patterns under real-world driving conditions, running in a EURO4 diesel vehicle and in a typical urban circuit in Madrid (Spain). Emission profiles were determined as a function of driving conditions. Source

Trapped fast particle destabilization of internal kink mode for the locally flattened q-profile with an inflection point

Energy Technology Data Exchange (ETDEWEB)

Wang, Xian-Qu [Institute of Fusion Science, School of Physical Science and Technology, Southwest Jiaotong University, Chengdu, Sichuan 610031 (China); Zhang, Rui-Bin; Meng, Guo [State Key Lab of Nuclear Physics and Technology, School of Physics, Peking University, Beijing 100871 (China)

2016-07-15

The destabilization of ideal internal kink modes by trapped fast particles in tokamak plasmas with a “shoulder”-like equilibrium current is investigated. It is found that energetic particle branch of the mode is unstable with the driving of fast-particle precession drifts and corresponds to a precessional fishbone. The mode with a low stability threshold is also more easily excited than the conventional precessional fishbone. This is different from earlier studies for the same equilibrium in which the magnetohydrodynamic (MHD) branch of the mode is stable. Furthermore, the stability and characteristic frequency of the mode are analyzed by solving the dispersion relation and comparing with the conventional fishbone. The results suggest that an equilibrium with a locally flattened q-profile, may be modified by localized current drive (or bootstrap current, etc.), is prone to the onset of the precessional fishbone branch of the mode.

Experimental studies on particle emissions from cruising ship, their characteristic properties, transformation and atmospheric lifetime in the marine boundary layer

Directory of Open Access Journals (Sweden)

A. Petzold

2008-05-01

Full Text Available Particle emissions from ship engines and their atmospheric transformation in the marine boundary layer (MBL were investigated in engine test bed studies and in airborne measurements of expanding ship plumes. During the test rig studies, detailed aerosol microphysical and chemical properties were measured in the exhaust gas of a serial MAN B&W seven-cylinder four-stroke marine diesel engine under various load conditions. The emission studies were complemented by airborne aerosol transformation studies in the plume of a large container ship in the English Channel using the DLR aircraft Falcon 20 E-5. Observations from emission studies and plume studies combined with a Gaussian plume dispersion model yield a consistent picture of particle transformation processes from emission to atmospheric processing during plume expansion. Particulate matter emission indices obtained from plume measurements are 8.8±1.0×10¹⁵(kg fuel⁻¹ by number for non-volatile particles and 174±43 mg (kg fuel⁻¹ by mass for Black Carbon (BC. Values determined for test rig conditions between 85 and 110% engine load are of similar magnitude. For the total particle number including volatile compounds no emission index can be derived since the volatile aerosol fraction is subject to rapid transformation processes in the plume. Ship exhaust particles occur in the size range D_p<0.3 μm, showing a bi-modal structure. The combustion particle mode is centred at modal diameters of 0.05 μm for raw emissions to 0.10 μm at a plume age of 1 h. The smaller-sized volatile particle mode is centred at D_p≤0.02 μm. From the decay of ship exhaust particle number concentrations in an expanding plume, a maximum plume life time of approx. 24 h is estimated for a well-mixed marine boundary layer.

Particle-in-cell studies of fast-ion slowing-down rates in cool tenuous magnetized plasma

Science.gov (United States)

Evans, Eugene S.; Cohen, Samuel A.; Welch, Dale R.

2018-04-01

We report on 3D-3V particle-in-cell simulations of fast-ion energy-loss rates in a cold, weakly-magnetized, weakly-coupled plasma where the electron gyroradius, ρe, is comparable to or less than the Debye length, λDe, and the fast-ion velocity exceeds the electron thermal velocity, a regime in which the electron response may be impeded. These simulations use explicit algorithms, spatially resolve ρe and λDe, and temporally resolve the electron cyclotron and plasma frequencies. For mono-energetic dilute fast ions with isotropic velocity distributions, these scaling studies of the slowing-down time, τs, versus fast-ion charge are in agreement with unmagnetized slowing-down theory; with an applied magnetic field, no consistent anisotropy between τs in the cross-field and field-parallel directions could be resolved. Scaling the fast-ion charge is confirmed as a viable way to reduce the required computational time for each simulation. The implications of these slowing down processes are described for one magnetic-confinement fusion concept, the small, advanced-fuel, field-reversed configuration device.

Fast-ion response to energetic-particle-driven MHD activity in Heliotron J

Energy Technology Data Exchange (ETDEWEB)

Kobayashi, S.; Yamamoto, S.; Mizuuchi, T.; Nagasaki, K.; Okada, H.; Minami, T.; Hanatani, K.; Konoshima, S.; Ohshima, S.; Toushi, K.; Sano, F. [Institute of Advanced Energy, Kyoto University, Gokasho, Uji (Japan); Nagaoka, K.; Suzuki, Y.; Takeiri, Y.; Yokoyama, M. [National Institute for Fusion Science, Toki, Gifu (Japan); Murakami, S. [Graduate School of Engineering, Kyoto University, Kyoto (Japan); Lee, H.Y.; Nakamura, Y.; Hosaka, K. [Graduate School of Energy Science, Kyoto University, Gokasho, Uji (Japan)

2010-08-15

In Heliotron J, low magnetic shear configuration, instabilities with frequency chirping in the frequency range of Alfven eigenmodes have been observed in tangentially injected neutral beam plasmas. These modes are induced by energetic-particle driven magnetohydrodynamic (MHD) instabilities such as global Alfven eigenmode or energetic particle mode. A hybrid directional Langmuir probe system has been installed into Heliotron J to investigate the response of fast-ion fluxes to the MHD modes. A high coherent response of the ion flux to the bursting modes has been observed not only by the co-directed probe but also by the counter-directed one. A linear correlation between the response of the co-directed ion flux and the mode amplitude has been found. The radial profile of the response of the co-directed ions has decreased with the minor radius and has not been obtained significantly outside last closed flux surface. These results indicate that the fast-ion response is due to a resonant convective oscillation. The ion flux response of the counter-directed probe has appeared in the growth phase of the mode burst. Its phase relation is different from that of co-directed one and magnetic probe located at the Heliotron J vacuum vessel. Two candidates of the detected ion flux of the counter-directed probe have been discussed. (copyright 2010 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

A fast sorting algorithm for a hypersonic rarefied flow particle simulation on the connection machine

Science.gov (United States)

Dagum, Leonardo

1989-01-01

The data parallel implementation of a particle simulation for hypersonic rarefied flow described by Dagum associates a single parallel data element with each particle in the simulation. The simulated space is divided into discrete regions called cells containing a variable and constantly changing number of particles. The implementation requires a global sort of the parallel data elements so as to arrange them in an order that allows immediate access to the information associated with cells in the simulation. Described here is a very fast algorithm for performing the necessary ranking of the parallel data elements. The performance of the new algorithm is compared with that of the microcoded instruction for ranking on the Connection Machine.

Energetic charged particle emission from hydrogen-loaded Pd and Ti cathodes and its enhancement by He-4 implantation

Energy Technology Data Exchange (ETDEWEB)

Lipson, A.G.; Miley, G.H. [University of Illinois at Urbana - Champaign, lL (United States); Lipson, A.G.; Lyakhov, B.F. [lnstitute of Physical Chemistry, The Russian Academy of Sciences, Moscow (Russian Federation); Roussetski, A.S. [P. N. Lebedev Physics Institute, The Russian Academy of Sciences Moscow (Russian Federation)

2006-07-01

In this paper, we demonstrate reproducible emissions of energetic alphas and protons appearing in an energy range where both cosmic ray interference and possible alpha emissions from contamination (e.g., radon) is assumed to be negligible. We also show that, {sup 4}He doping of Pd and Ti cathodes leads to a significant enhancement of the energetic charged particles emission (ECPE). This measurement of the emissions of energetic (MeV) particles, in a region of low background interference plus their enhancement by {sup 4}He doping provides very strong support for the existence of LENR processes in the crystalline lattice of deuterated metals. (authors)

Explaining global surface aerosol number concentrations in terms of primary emissions and particle formation

Science.gov (United States)

Spracklen, D. V.; Carslaw, K. S.; Merikanto, J.; Mann, G. W.; Reddington, C. L.; Pickering, S.; Ogren, J. A.; Andrews, E.; Baltensperger, U.; Weingartner, E.; Boy, M.; Kulmala, M.; Laakso, L.; Lihavainen, H.; Kivekäs, N.; Komppula, M.; Mihalopoulos, N.; Kouvarakis, G.; Jennings, S. G.; O'Dowd, C.; Birmili, W.; Wiedensohler, A.; Weller, R.; Gras, J.; Laj, P.; Sellegri, K.; Bonn, B.; Krejci, R.; Laaksonen, A.; Hamed, A.; Minikin, A.; Harrison, R. M.; Talbot, R.; Sun, J.

2010-05-01

We synthesised observations of total particle number (CN) concentration from 36 sites around the world. We found that annual mean CN concentrations are typically 300-2000 cm-3 in the marine boundary layer and free troposphere (FT) and 1000-10 000 cm-3 in the continental boundary layer (BL). Many sites exhibit pronounced seasonality with summer time concentrations a factor of 2-10 greater than wintertime concentrations. We used these CN observations to evaluate primary and secondary sources of particle number in a global aerosol microphysics model. We found that emissions of primary particles can reasonably reproduce the spatial pattern of observed CN concentration (R2=0.46) but fail to explain the observed seasonal cycle (R2=0.1). The modeled CN concentration in the FT was biased low (normalised mean bias, NMB=-88%) unless a secondary source of particles was included, for example from binary homogeneous nucleation of sulfuric acid and water (NMB=-25%). Simulated CN concentrations in the continental BL were also biased low (NMB=-74%) unless the number emission of anthropogenic primary particles was increased or a mechanism that results in particle formation in the BL was included. We ran a number of simulations where we included an empirical BL nucleation mechanism either using the activation-type mechanism (nucleation rate, J, proportional to gas-phase sulfuric acid concentration to the power one) or kinetic-type mechanism (J proportional to sulfuric acid to the power two) with a range of nucleation coefficients. We found that the seasonal CN cycle observed at continental BL sites was better simulated by BL particle formation (R2=0.3) than by increasing the number emission from primary anthropogenic sources (R2=0.18). The nucleation constants that resulted in best overall match between model and observed CN concentrations were consistent with values derived in previous studies from detailed case studies at individual sites. In our model, kinetic and activation

Comparative evaluation of GHG emissions from the use of Miscanthus for bio-hydrocarbon production via fast pyrolysis and bio-oil upgrading

International Nuclear Information System (INIS)

Shemfe, Mobolaji B.; Whittaker, Carly; Gu, Sai; Fidalgo, Beatriz

2016-01-01

Highlights: • GHG emissions from the upgrading of pyrolysis-derived bio-oil is quantified.. • Soil organic carbon sequestration rate had a significant effect on GHG emission. • Increasing plant scale could improve the environmental performance of the system. • Nitrogen to the pyrolysis reactor had significant impact on GHG emissions. - Abstract: This study examines the GHG emissions associated with producing bio-hydrocarbons via fast pyrolysis of Miscanthus. The feedstock is then upgraded to bio-oil products via hydroprocessing and zeolite cracking. Inventory data for this study were obtained from current commercial cultivation practices of Miscanthus in the UK and state-of-the-art process models developed in Aspen Plus®. The system boundary considered spans from the cultivation of Miscanthus to conversion of the pyrolysis-derived bio-oil into bio-hydrocarbons up to the refinery gate. The Miscanthus cultivation subsystem considers three scenarios for soil organic carbon (SOC) sequestration rates. These were assumed as follows: (i) excluding (SOC), (ii) low SOC and (iii) high (SOC) for best and worst cases. Overall, Miscanthus cultivation contributed moderate to negative values to GHG emissions, from analysis of excluding SOC to high SOC scenarios. Furthermore, the rate of SOC in the Miscanthus cultivation subsystem has significant effects on total GHG emissions. Where SOC is excluded, the fast pyrolysis subsystem shows the highest positive contribution to GHG emissions, while the credit for exported electricity was the main ‘negative’ GHG emission contributor for both upgrading pathways. Comparison between the bio-hydrocarbons produced from the two upgrading routes and fossil fuels indicates GHG emission savings between 68% and 87%. Sensitivity analysis reveals that bio-hydrocarbon yield and nitrogen gas feed to the fast pyrolysis reactor are the main parameters that influence the total GHG emissions for both pathways.

Emissions from carpet combustion in a pilot-scale rotary kiln: comparison with coal and particle-board combustion

Energy Technology Data Exchange (ETDEWEB)

Stephanie Lucero Konopa; James A. Mulholland; Matthew J. Realff; Paul M. Lemieux [Georgia Institute of Technology, Atlanta, GA (United States). School of Civil and Environmental Engineering

2008-08-15

The use of post-consumer carpet as a potential fuel substitute in cement kilns and other high-temperature processes is being considered to address the problem of huge volumes of carpet waste and the opportunity of waste-to-energy recovery. Carpet represents a high volume waste stream, provides high energy value, and contains other recoverable materials for the production of cement. This research studied the emission characteristics of burning 0.46-kg charges of chopped nylon carpet squares, pulverized coal, and particle-board pellets in a pilot-scale natural gas-fired rotary kiln. Carpet was tested with different amounts of water added. Emissions of oxygen, carbon dioxide, nitric oxide (NO), sulfur dioxide (SO{sub 2}), carbon monoxide (CO), and total hydrocarbons and temperatures were continuously monitored. It was found that carpet burned faster and more completely than coal and particle board, with a rapid volatile release that resulted in large and variable transient emission peaks. NO emissions from carpet combustion ranged from 0.06 to 0.15 g/MJ and were inversely related to CO emissions. Carpet combustion yielded higher NO emissions than coal and particleboard combustion, consistent with its higher nitrogen content. S{sub 2} emissions were highest for coal combustion, consistent with its higher sulfur content than carpet or particle board. Adding water to carpet slowed its burn time and reduced variability in the emission transients, reducing the CO peak but increasing NO emissions. Results of this study indicate that carpet waste can be used as an effective alternative fuel, with the caveats that it might be necessary to wet carpet or chop it finely to avoid excessive transient puff emissions due to its high volatility compared with other solid fuels, and that controlled mixing of combustion air might be used to control NO emissions from nylon carpet. 13 refs., 5 figs., 1 tab.

A source-independent empirical correction procedure for the fast mobility and engine exhaust particle sizers

Science.gov (United States)

Zimmerman, Naomi; Jeong, Cheol-Heon; Wang, Jonathan M.; Ramos, Manuel; Wallace, James S.; Evans, Greg J.

2015-01-01

The TSI Fast Mobility Particle Sizer (FMPS) and Engine Exhaust Particle Sizer (EEPS) provide size distributions for 6-560 nm particles with a time resolution suitable for characterizing transient particle sources; however, the accuracy of these instruments can be source dependent, due to influences of particle morphology. The aim of this study was to develop a source-independent correction protocol for the FMPS and EEPS. The correction protocol consists of: (1) broadening the >80 nm size range of the distribution to account for under-sizing by the FMPS and EEPS; (2) applying an existing correction protocol in the 8-93 nm size range; and (3) dividing each size bin by the ratio of total concentration measured by the FMPS or EEPS and a water-based Condensation Particle Counter (CPC) as a surrogate scaling factor to account for particle morphology. Efficacy of the correction protocol was assessed for three sources: urban ambient air, diluted gasoline direct injection engine exhaust, and diluted diesel engine exhaust. Linear regression against a reference instrument, the Scanning Mobility Particle Sizer (SMPS), before and after applying the correction protocol demonstrated that the correction ensured agreement within 20%.

[Emission characteristics of fine particles from grate firing boilers].

Science.gov (United States)

Wang, Shu-Xiao; Zhao, Xiu-Juan; Li, Xing-Hua; Wei, Wei; Hao, Ji-Ming

2009-04-15

Grate firing boilers are the main type of Chinese industrial boilers, which accounts for 85% of the industrial boilers and is one of the most important emission sources of primary air pollutants in China. In this study, five boilers in three cities were selected and tested to measure the emission characteristics of PM2.5, and gaseous pollutants were applied by a compact dilution sampling system, which was developed for this field study. Results showed that particles mass size distributions for the five industrial boilers presented single peak or double peak, former peaks near 0.14 microm and the later peaks after 1.0 microm; the cyclone dust remover and wet scrubber dust remover had effective removal efficiencies not only to PM2.5, but also to PM1.0; and under the condition of same control techniques, grate firing boiler with high capacity has less PM2.5 emission than the boiler with low capacity. In the PM2.5 collected from flue gases, SO4(2-) was the most abundant ion, accounted for 20%-40% of the PM2.5; and C was the most abundant element (7.5%-31.8%), followed by S (8.4%-18.7%). Carbon balance method was applied to calculate the emission factors of these pollutants. The emission factors of PM2.5, NO, and SO2 were in the range of 0.046-0.486 g x kg(-1), 1.63-2.47 g x kg(-1), 1.35-9.95 g x kg(-1) respectively. The results are useful for the emission inventory development of industrial boilers and the source analysis of PM2.5 in atmospheric environment.

Signal enhancement of neutral He emission lines by fast electron bombardment of laser-induced He plasma

Directory of Open Access Journals (Sweden)

Hery Suyanto

2016-08-01

Full Text Available A time-resolved spectroscopic study is performed on the enhancement signals of He gas plasma emission using nanosecond (ns and picosecond (ps lasers in an orthogonal configuration. The ns laser is used for the He gas plasma generation and the ps laser is employed for the ejection of fast electrons from a metal target, which serves to excite subsequently the He atoms in the plasma. The study is focused on the most dominant He I 587.6 nm and He I 667.8 nm emission lines suggested to be responsible for the He-assisted excitation (HAE mechanism. The time-dependent intensity enhancements induced by the fast electrons generated with a series of delayed ps laser ablations are deduced from the intensity time profiles of both He emission lines. The results clearly lead to the conclusion that the metastable excited triplet He atoms are actually the species overwhelmingly produced during the recombination process in the ns laser-induced He gas plasma. These metastable He atoms are believed to serve as the major energy source for the delayed excitation of analyte atoms in ns laser-induced breakdown spectroscopy (LIBS using He ambient gas.

Signal enhancement of neutral He emission lines by fast electron bombardment of laser-induced He plasma

Energy Technology Data Exchange (ETDEWEB)

Suyanto, Hery [Department of Physics, Faculty of Mathematics and Natural Sciences, Udayana University, Kampus Bukit Jimbaran, Denpasar 80361, Bali (Indonesia); Pardede, Marincan [Department of Electrical Engineering, University of Pelita Harapan, 1100 M.H. Thamrin Boulevard, Lippo Village, Tangerang 15811 (Indonesia); Hedwig, Rinda [Department of Computer Engineering, Bina Nusantara University, 9 K.H. Syahdan, Jakarta 14810 (Indonesia); Marpaung, Alion Mangasi [Department of Physics, Faculty of Mathematics and Natural Sciences, Jakarta State University, Rawamangun, Jakarta 12440 (Indonesia); Ramli, Muliadi [Department of Chemistry, Faculty of Mathematics and Natural Sciences, Syiah Kuala University, Darussalam, Banda Aceh 23111, NAD (Indonesia); Lie, Tjung Jie; Kurniawan, Koo Hendrik, E-mail: kurnia18@cbn.net.id [Research Center of Maju Makmur Mandiri Foundation, 40 Srengseng Raya, Kembangan, Jakarta Barat 11630 (Indonesia); Abdulmadjid, Syahrun Nur [Department of Physics, Faculty of Mathematics and Natural Sciences, Syiah Kuala University, Darussalam, Banda Aceh 23111, NAD (Indonesia); Tjia, May On [Research Center of Maju Makmur Mandiri Foundation, 40 Srengseng Raya, Kembangan, Jakarta Barat 11630 (Indonesia); Physics of Magnetism and Photonics Group, Faculty of Mathematics and Natural Sciences, Bandung Institute of Technology, 10 Ganesha,Bandung 40132 (Indonesia); Kagawa, Kiichiro [Research Center of Maju Makmur Mandiri Foundation, 40 Srengseng Raya, Kembangan, Jakarta Barat 11630 (Indonesia); Fukui Science Education Academy, Takagi Chuo 2 chome, Fukui 910-0804 (Japan)

2016-08-15

A time-resolved spectroscopic study is performed on the enhancement signals of He gas plasma emission using nanosecond (ns) and picosecond (ps) lasers in an orthogonal configuration. The ns laser is used for the He gas plasma generation and the ps laser is employed for the ejection of fast electrons from a metal target, which serves to excite subsequently the He atoms in the plasma. The study is focused on the most dominant He I 587.6 nm and He I 667.8 nm emission lines suggested to be responsible for the He-assisted excitation (HAE) mechanism. The time-dependent intensity enhancements induced by the fast electrons generated with a series of delayed ps laser ablations are deduced from the intensity time profiles of both He emission lines. The results clearly lead to the conclusion that the metastable excited triplet He atoms are actually the species overwhelmingly produced during the recombination process in the ns laser-induced He gas plasma. These metastable He atoms are believed to serve as the major energy source for the delayed excitation of analyte atoms in ns laser-induced breakdown spectroscopy (LIBS) using He ambient gas.

Ion desorption induced by charged particle beams: mechanisms and mass spectroscopy

International Nuclear Information System (INIS)

Silveira, E.F. da; Schweikert, E.A.

1988-01-01

Surface analysis, through desorption, induced by fast particles, is presented and discussed. The stopping of projectils is essentially made by collisions with the target electrons. The desorbed particles are generally emmited with kinetic energy from 0.1 to 20 eV. Mass, charge, velocity and emission angle give information about the surface components, its structure as well as beam-solid interaction processes. Time-of-flight mass spectroscopy of desorbed ions, determine the mass of organic macromolecules and biomolecules. (A.C.A.S.) [pt

CHARGED PARTICLE MOTION IN AN EXPLOSIVELY GENERATED IONIZING SHOCK

International Nuclear Information System (INIS)

Boswell, Christopher J.; O'Connor, Patrick D.

2009-01-01

Different aspects of the plasma generated in a gas contained in a tube due to detonation of a small explosive charge located at one end of the tube are presented. The motion of the charged particles within the plasma is monitored using Rogowski coils. Using time-resolved emission spectroscopy the temperature and species in the detonation products and compressed gas behind the shock wave are recorded. From the spectral lines of the emission profiles the temperatures and electron density were evaluated to be in the vicinity of 7,000 K and 5x10 22 m -3 . An ultra fast wave traveling down the guide tube ahead of the hydrodynamic shock and causing any charged particles there to move fast enough to be detected by the Rogowski coils was recorded. From the measurements the phase velocity of the wave was calculated at 525 km/s when krypton filled the tube, and 1300 km/s in the case of argon. The temperature and density measurements are consistent with the data reported in the literature for similar tests. The electrostatic pulse measurements are a new phenomena not previously observed.

Fast-scanning heterodyne receiver for measurement of the electron cyclotron emission from high-temperature plasmas

International Nuclear Information System (INIS)

Efthimion, P.C.; Arunasalam, V.; Bitzer, R.; Campbell, L.; Hosea, J.C.

1979-03-01

A fast-scanning heterodyne receiver was developed that measures the fundamental cyclotron emission from the PLT plasma and thus ascertains the time evolution of the electron temperature profile. The receiver scans 60 to 90 GHz every 10 milliseconds and is interfaced to a computer for completely automated calibrated temperature measurements

Active and fast particle driven Alfvén eigenmodes in Alcator C-Moda)

Science.gov (United States)

Snipes, J. A.; Basse, N.; Boswell, C.; Edlund, E.; Fasoli, A.; Gorelenkov, N. N.; Granetz, R. S.; Lin, L.; Lin, Y.; Parker, R.; Porkolab, M.; Sears, J.; Sharapov, S.; Tang, V.; Wukitch, S.

2005-05-01

Alfvén eigenmodes (AEs) are studied to assess their stability in high density reactor relevant regimes where Ti≈Te and as a diagnostic tool. Stable AEs are excited with active magnetohydrodynamics antennas in the range of the expected AE frequency. Toroidal Alfvén eigenmode (TAE) damping rates between 0.5%<γ/ω<4.5% have been observed in diverted and limited Ohmic plasmas. Unstable AEs are excited with a fast ion tail driven by H minority ion cyclotron radio frequency (ICRF) heating with electron densities in the range of n¯e=0.5-2×1020m-3. Energetic particle modes or TAEs have been observed to decrease in frequency and mode number with time up to a large sawtooth collapse, indicating the role fast particles play in stabilizing sawteeth. In the current rise phase, unstable modes with frequencies that increase rapidly with time are observed with magnetic pick-up coils at the wall and phase contrast imaging density fluctuation measurements in the core. Modeling of these modes constrains the calculated safety factor profile to be very flat or with slightly reversed shear. AEs are found to be more stable for an inboard than for central or outboard ICRF resonances in qualitative agreement with modeling.

Take-off engine particle emission indices for in-service aircraft at Los Angeles International Airport

Science.gov (United States)

Moore, Richard H.; Shook, Michael A.; Ziemba, Luke D.; Digangi, Joshua P.; Winstead, Edward L.; Rauch, Bastian; Jurkat, Tina; Thornhill, Kenneth L.; Crosbie, Ewan C.; Robinson, Claire; Shingler, Taylor J.; Anderson, Bruce E.

2017-12-01

We present ground-based, advected aircraft engine emissions from flights taking off at Los Angeles International Airport. 275 discrete engine take-off plumes were observed on 18 and 25 May 2014 at a distance of 400 m downwind of the runway. CO2 measurements are used to convert the aerosol data into plume-average emissions indices that are suitable for modelling aircraft emissions. Total and non-volatile particle number EIs are of order 1016-1017 kg-1 and 1014-1016 kg-1, respectively. Black-carbon-equivalent particle mass EIs vary between 175-941 mg kg-1 (except for the GE GEnx engines at 46 mg kg-1). Aircraft tail numbers recorded for each take-off event are used to incorporate aircraft- and engine-specific parameters into the data set. Data acquisition and processing follow standard methods for quality assurance. A unique aspect of the data set is the mapping of aerosol concentration time series to integrated plume EIs, aircraft and engine specifications, and manufacturer-reported engine emissions certifications. The integrated data enable future studies seeking to understand and model aircraft emissions and their impact on air quality.

Take-off engine particle emission indices for in-service aircraft at Los Angeles International Airport.

Science.gov (United States)

Moore, Richard H; Shook, Michael A; Ziemba, Luke D; DiGangi, Joshua P; Winstead, Edward L; Rauch, Bastian; Jurkat, Tina; Thornhill, Kenneth L; Crosbie, Ewan C; Robinson, Claire; Shingler, Taylor J; Anderson, Bruce E

2017-12-19

We present ground-based, advected aircraft engine emissions from flights taking off at Los Angeles International Airport. 275 discrete engine take-off plumes were observed on 18 and 25 May 2014 at a distance of 400 m downwind of the runway. CO 2 measurements are used to convert the aerosol data into plume-average emissions indices that are suitable for modelling aircraft emissions. Total and non-volatile particle number EIs are of order 10 16 -10 17 kg -1 and 10 14 -10 16 kg -1 , respectively. Black-carbon-equivalent particle mass EIs vary between 175-941 mg kg -1 (except for the GE GEnx engines at 46 mg kg -1 ). Aircraft tail numbers recorded for each take-off event are used to incorporate aircraft- and engine-specific parameters into the data set. Data acquisition and processing follow standard methods for quality assurance. A unique aspect of the data set is the mapping of aerosol concentration time series to integrated plume EIs, aircraft and engine specifications, and manufacturer-reported engine emissions certifications. The integrated data enable future studies seeking to understand and model aircraft emissions and their impact on air quality.

14th International Conference on Particle Induced X-ray Emission ("PIXE 2015")

Science.gov (United States)

Przybyłowicz, Wojciech Józef; Pineda-Vargas, Carlos

2015-11-01

This special issue of Nuclear Instruments and Methods in Physics Research B contains the proceedings of the 14th International Conference on Particle Induced X-ray Emission ("PIXE 2015") that was held in Somerset West (South Africa) from 25th February to 3rd March 2015.

Extent of pyrolysis impacts on fast pyrolysis biochar properties.

Science.gov (United States)

Brewer, Catherine E; Hu, Yan-Yan; Schmidt-Rohr, Klaus; Loynachan, Thomas E; Laird, David A; Brown, Robert C

2012-01-01

A potential concern about the use of fast pyrolysis rather than slow pyrolysis biochars as soil amendments is that they may contain high levels of bioavailable C due to short particle residence times in the reactors, which could reduce the stability of biochar C and cause nutrient immobilization in soils. To investigate this concern, three corn ( L.) stover fast pyrolysis biochars prepared using different reactor conditions were chemically and physically characterized to determine their extent of pyrolysis. These biochars were also incubated in soil to assess their impact on soil CO emissions, nutrient availability, microorganism population growth, and water retention capacity. Elemental analysis and quantitative solid-state C nuclear magnetic resonance spectroscopy showed variation in O functional groups (associated primarily with carbohydrates) and aromatic C, which could be used to define extent of pyrolysis. A 24-wk incubation performed using a sandy soil amended with 0.5 wt% of corn stover biochar showed a small but significant decrease in soil CO emissions and a decrease in the bacteria:fungi ratios with extent of pyrolysis. Relative to the control soil, biochar-amended soils had small increases in CO emissions and extractable nutrients, but similar microorganism populations, extractable NO levels, and water retention capacities. Corn stover amendments, by contrast, significantly increased soil CO emissions and microbial populations, and reduced extractable NO. These results indicate that C in fast pyrolysis biochar is stable in soil environments and will not appreciably contribute to nutrient immobilization. Copyright © by the American Society of Agronomy, Crop Science Society of America, and Soil Science Society of America, Inc.

Reduction of particle emissions from light duty vehicles and from taxies; Reduktion af partikelelemissioner fra varebiler og taxier

Energy Technology Data Exchange (ETDEWEB)

Nielsen, Johan; Henriques, M.; Weibel, T.G. [TetraPlan A/S (Denmark)

2006-11-03

This project, 'Reduction of particle emissions from light duty vehicles and from taxies', analyses different strategies to reduce the particle emission, their effect for particle emissions, and the resulting cost for the society and for the companies. The project describes the EU regulation of emissions, the possibilities of reducing the emissions via special requirements in environmental zones and the Danish taxation of light duty vehicles. Further, the project includes interviews with owners of light duty vehicles and taxies and also with Danish producers of particle filters. The strategies analysed in the scenarios include: 1) Promotion of particle filters; 2) Shift from diesel to gasoline and; 3) Downsizing. The effects for particle emissions and for mortality are described. Further, the costs and benefits for the society and the cost for the companies are evaluated. The effects of the scenarios are analysed, both for initiatives implemented at a national level and for implementation in an environmental zone in the municipality of Copenhagen. The main results are that the socioeconomic benefits in the year 2012 are greater than the costs, if taxis and light duty vehicles have filters installed and if they are driving in the Copenhagen area. For light duty vehicles it is only profitable, if the prices of the filters fall to the price level that is expected in the future in the study. Further, the analysis shows that for light duty vehicles and taxies driving all over the country, the socioeconomic benefits achieved by installing particle filters are too small to cover the costs. The analysis shows that it is also profitable socio-economically to change from diesel to petrol for light duty vehicles and for taxies (except taxies driving nationally). The analysis is based on the producer prices including the general net tax level, while the specific taxes are not included. From the point of view of the companies it is not profitable to change to petrol

Indoor emission, dispersion and exposure of total particle-bound polycyclic aromatic hydrocarbons during cooking

Science.gov (United States)

Gao, Jun; Jian, Yating; Cao, Changsheng; Chen, Lei; Zhang, Xu

2015-11-01

Cooking processes highly contribute to indoor polycyclic aromatic hydrocarbon (PAH) pollution. High molecular weight and potentially carcinogenic PAHs are generally found attached to small particles, i.e., particulate phase PAHs (PPAHs). Due to the fact that indoor particle dynamics have been clear, describing the indoor dynamics of cooking-generated PPAHs within a specific time span is possible. This paper attempted to quantify the dynamic emission rate, simultaneous spatial dispersion and individual exposure of PPAHs using a cooking source. Experiments were conducted in a real-scale kitchen chamber to elucidate the time-resolved emission and effect of edible oil temperature and mass. Numerical simulations based on indoor particle dynamics were performed to obtain the spatial dispersion and individual inhalation intake of PPAHs under different emission and ventilation conditions. The present work examined the preheating cooking stage, at which edible oil is heated up to beyond its smoke point. The dynamic emission rate peak point occurred much earlier than the oil heating temperature. The total PPAH emission ranged from 2258 to 6578 ng upon heating 40-85 g of edible oil. The overall intake fraction by an individual within a period of 10 min, including 3 min for heating and 7 min for natural cooling, was generally ∼1/10,000. An important outcome of this work was that the overall intake fraction could be represented by multiplying the range hood escape efficiency by the inhalation-to-ventilation rate ratio, which would be no greater than the same ratio. The methodology and results of this work were extendible for the number-based assessment of PPAHs. This work is expected to help us understand the health risks due to inhalation exposure to cooking-generated PPAHs in the kitchen.

Effect of compression ratio, nozzle opening pressure, engine load, and butanol addition on nanoparticle emissions from a non-road diesel engine.

Science.gov (United States)

Maurya, Rakesh Kumar; Saxena, Mohit Raj; Rai, Piyush; Bhardwaj, Aashish

2018-05-01

Currently, diesel engines are more preferred over gasoline engines due to their higher torque output and fuel economy. However, diesel engines confront major challenge of meeting the future stringent emission norms (especially soot particle emissions) while maintaining the same fuel economy. In this study, nanosize range soot particle emission characteristics of a stationary (non-road) diesel engine have been experimentally investigated. Experiments are conducted at a constant speed of 1500 rpm for three compression ratios and nozzle opening pressures at different engine loads. In-cylinder pressure history for 2000 consecutive engine cycles is recorded and averaged data is used for analysis of combustion characteristics. An electrical mobility-based fast particle sizer is used for analyzing particle size and mass distributions of engine exhaust particles at different test conditions. Soot particle distribution from 5 to 1000 nm was recorded. Results show that total particle concentration decreases with an increase in engine operating loads. Moreover, the addition of butanol in the diesel fuel leads to the reduction in soot particle concentration. Regression analysis was also conducted to derive a correlation between combustion parameters and particle number emissions for different compression ratios. Regression analysis shows a strong correlation between cylinder pressure-based combustion parameters and particle number emission.

Eddy covariance measurements and parameterisation of traffic related particle emissions in an urban environment

Directory of Open Access Journals (Sweden)

E. M. Mårtensson

2006-01-01

Full Text Available Urban aerosol sources are important due to the health effects of particles and their potential impact on climate. Our aim has been to quantify and parameterise the urban aerosol source number flux F (particles m−2 s−1, in order to help improve how this source is represented in air quality and climate models. We applied an aerosol eddy covariance flux system 118.0 m above the city of Stockholm. This allowed us to measure the aerosol number flux for particles with diameters >11 nm. Upward source fluxes dominated completely over deposition fluxes in the collected dataset. Therefore, the measured fluxes were regarded as a good approximation of the aerosol surface sources. Upward fluxes were parameterised using a traffic activity (TA database, which is based on traffic intensity measurements. The footprint (area on the surface from which sources and sinks affect flux measurements, located at one point in space of the eddy system covered road and building construction areas, forests and residential areas, as well as roads with high traffic density and smaller streets. We found pronounced diurnal cycles in the particle flux data, which were well correlated with the diurnal cycles in traffic activities, strongly supporting the conclusion that the major part of the aerosol fluxes was due to traffic emissions. The emission factor for the fleet mix in the measurement area EFfm=1.4±0.1×1014 veh−1 km−1 was deduced. This agrees fairly well with other studies, although this study has an advantage of representing the actual effective emission from a mixed vehicle fleet. Emission from other sources, not traffic related, account for a F0=15±18×106 m−2 s−1. The urban aerosol source flux can then be written as F=EFfmTA+F0. In a second attempt to find a parameterisation, the friction velocity U* normalised with the average friction velocity has been included, F=EF . This parameterisation results in a somewhat reduced emission factor, 1.3×1014 veh�

Importance of the (n,gamma) Cm-247 Evaluation on Neutron Emission in Fast Reactor Fuel Cycle Analysis

International Nuclear Information System (INIS)

Benoit Forget; Mehdi Asgari; Rodolfo M. Ferrer

2007-01-01

As part of the GNEP program, it is envisioned to build a fast reactor for the transmutation of minor actinides. The spent nuclear fuel from the current fleet of light water reactors would be recycled, the current baseline is the UREX+1a process, and would act as a feed for the fast reactor. As the fuel is irradiated in a fast reactor a certain quantity of minor actinides would thus build up in the fuel stream creating possible concerns with the neutron emission of these minor actinides for fuel transportation, handling and fabrication. Past neutronic analyses had not tracked minor actinides above Cm-246 in the transmutation chain, because of the small influence on the overall reactor performance and cycle parameters. However, when trying to quantify the neutron emission from the recycled fuel with high minor actinide content, these higher isotopes play an essential role and should be included in the analysis. In this paper, the influence of tracking these minor actinides on the calculated neutron emission is presented. Also presented is the particular influence of choosing a different evaluated cross section data set to represent the minor actinides above Cm-246. The first representation uses the cross-sections provided by MC2-2 for all isotopes, while the second representation uses infinitely diluted ENDF/BVII.0 cross-sections for Cm-247 to Cf-252 and MC2-2 for all other isotopes

Particle correlation based measurement of the mean time between the deuteron and proton emissions

International Nuclear Information System (INIS)

Ghisalberti, C.; Lebrun, C.; Sezac, L.; Ardouin, D.; Erazmus, B.; Eudes, P.; Ghuilbault, F.; Lautridou, P.; Rahmani, J.A.; Reposeur, T.; Chbihi, A.; Galin, J.; Guerreau, D.; Morjean, M.; Peghaire, A.; Lednicky, R.; Pluta, J.; Quebert, J.; Siemssen, R.

1997-01-01

Proton-deuteron correlations at small relative momenta have been measured with the reaction 208 Pb + 93 Nb at 29 MeV per nucleon at GANIL using the ORION neutron calorimeter. By selecting the proton-deuteron pairs according to the angle between their relative velocity and the pair center of mass velocity of the emitting source one can determine the average value of the time delay between the emission of these particles. The results reported in this paper for the first time at GANIL energies agree with the values published before in the literature i.e. 600 and 1500 fm/c for deuteron and proton emission times, respectively, as obtained in the reactions Ar + Ag at E/A = 17 MeV. At higher energies measurements with a B.U.U. calorimeter recording the collisions 14 N + 27 Al at E/A = 75 MeV show that in this case the proton emission begins at 15 fm/c and decreases slowly in time, while the deuterons are emitted at 50 fm/c and present a steep falling. This result agrees with a negative average value of d - t p >. Thus, the method presented in this report for determining the order of emission is of great interest for checking the theoretical description of the particle emission all the way in the collision dynamical process

Emissions from Ethanol-Gasoline Blends: A Single Particle Perspective

Directory of Open Access Journals (Sweden)

Peter H. McMurry

2011-06-01

Full Text Available Due to its agricultural origin and function as a fuel oxygenate, ethanol is being promoted as an alternative biomass-based fuel for use in spark ignition engines, with mandates for its use at state and regional levels. While it has been established that the addition of ethanol to a fuel reduces the particulate mass concentration in the exhaust, little attention has been paid to changes in the physicochemical properties of the emitted particles. In this work, a dynamometer-mounted GM Quad-4 spark ignition engine run without aftertreatment at 1,500 RPM and 100% load was used with four different fuel blends, containing 0, 20, 40 and 85 percent ethanol in gasoline. This allowed the effects of the fuel composition to be isolated from other effects. Instrumentation employed included two Aerosol Time-of-Flight Mass Spectrometers covering different size ranges for analysis of single particle composition, an Aethalometer for black carbon, a Scanning Mobility Particle Sizer for particle size distributions, a Photoelectric Aerosol Sensor for particle-bound polycyclic aromatic hydrocarbon (PAH species and gravimetric filter measurements for particulate mass concentrations. It was found that, under the conditions investigated here, additional ethanol content in the fuel changes the particle size distribution, especially in the accumulation mode, and decreases the black carbon and total particulate mass concentrations. The molecular weight distribution of the PAHs was found to decrease with added ethanol. However, PAHs produced from higher ethanol-content fuels are associated with NO2− (m/z—46 in the single-particle mass spectra, indicating the presence of nitro-PAHs. Compounds associated with the gasoline (e.g., sulfur-containing species are diminished due to dilution as ethanol is added to the fuel relative to those associated with the lubricating oil (e.g., calcium, zinc, phosphate in the single particle spectra. These changes have potential

The future of airborne sulfur-containing particles in the absence of fossil fuel sulfur dioxide emissions.

Science.gov (United States)

Perraud, Véronique; Horne, Jeremy R; Martinez, Andrew S; Kalinowski, Jaroslaw; Meinardi, Simone; Dawson, Matthew L; Wingen, Lisa M; Dabdub, Donald; Blake, Donald R; Gerber, R Benny; Finlayson-Pitts, Barbara J

2015-11-03

Sulfuric acid (H2SO4), formed from oxidation of sulfur dioxide (SO2) emitted during fossil fuel combustion, is a major precursor of new airborne particles, which have well-documented detrimental effects on health, air quality, and climate. Another precursor is methanesulfonic acid (MSA), produced simultaneously with SO2 during the atmospheric oxidation of organosulfur compounds (OSCs), such as dimethyl sulfide. In the present work, a multidisciplinary approach is used to examine how contributions of H2SO4 and MSA to particle formation will change in a large coastal urban area as anthropogenic fossil fuel emissions of SO2 decline. The 3-dimensional University of California Irvine-California Institute of Technology airshed model is used to compare atmospheric concentrations of gas phase MSA, H2SO4, and SO2 under current emissions of fossil fuel-associated SO2 and a best-case futuristic scenario with zero fossil fuel sulfur emissions. Model additions include results from (i) quantum chemical calculations that clarify the previously uncertain gas phase mechanism of formation of MSA and (ii) a combination of published and experimental estimates of OSC emissions, such as those from marine, agricultural, and urban processes, which include pet waste and human breath. Results show that in the zero anthropogenic SO2 emissions case, particle formation potential from H2SO4 will drop by about two orders of magnitude compared with the current situation. However, particles will continue to be generated from the oxidation of natural and anthropogenic sources of OSCs, with contributions from MSA and H2SO4 of a similar order of magnitude. This could be particularly important in agricultural areas where there are significant sources of OSCs.

Enhancement of single particle rare earth doped NaYF4: Yb, Er emission with a gold shell

International Nuclear Information System (INIS)

Li, Ling; Green, Kory; Hallen, Hans; Lim, Shuang Fang

2015-01-01

Upconversion of infrared light to visible light has important implications for bioimaging. However, the small absorption cross-section of rare earth dopants has limited the efficiency of these anti-Stokes nanomaterials. We present enhanced excitation absorption and single particle fluorescent emission of sodium yttrium fluoride, NaYF 4 : Yb, Er based upconverting nanoparticles coated with a gold nanoshell through surface plasmon resonance. The single gold-shell coated nanoparticles show enhanced absorption in the near infrared, enhanced total emission intensity, and increased green relative to red emission. We also show differences in enhancement between single and aggregated gold shell nanoparticles. The surface plasmon resonance of the gold-shell coated nanoparticle is shown to be dependent on the shell thickness. In contrast to other reported results, our single particle experimental observations are corroborated by finite element calculations that show where the green/red emission enhancement occurs, and what portion of the enhancement is due to electromagnetic effects. We find that the excitation enhancement and green/red emission ratio enhancement occurs at the corners and edges of the doped emissive core. (paper)

Fast detector for triggering on charged particle multiplicity for relativistic nucleus-nucleus collisions

International Nuclear Information System (INIS)

Agakishiev, G.; Man'yakov, P.K.; Drees, A.

1997-01-01

The simple and fast detector of charged particle multiplicity for relativistic nucleus-nucleus collision studies is performed. The multiplicity detector has been designed for the first level trigger of the CERES/NA45 experiment to study Pb-Au collisions at CERN SPS energies. The detector has allowed a realization of the 40 ns trigger for selection of events with definite impact parameter. The construction, operation characteristics, method of calibration, and testing results are described in detail

Explaining global surface aerosol number concentrations in terms of primary emissions and particle formation

Directory of Open Access Journals (Sweden)

D. V. Spracklen

2010-05-01

Full Text Available We synthesised observations of total particle number (CN concentration from 36 sites around the world. We found that annual mean CN concentrations are typically 300–2000 cm⁻³ in the marine boundary layer and free troposphere (FT and 1000–10 000 cm⁻³ in the continental boundary layer (BL. Many sites exhibit pronounced seasonality with summer time concentrations a factor of 2–10 greater than wintertime concentrations. We used these CN observations to evaluate primary and secondary sources of particle number in a global aerosol microphysics model. We found that emissions of primary particles can reasonably reproduce the spatial pattern of observed CN concentration (R²=0.46 but fail to explain the observed seasonal cycle (R²=0.1. The modeled CN concentration in the FT was biased low (normalised mean bias, NMB=−88% unless a secondary source of particles was included, for example from binary homogeneous nucleation of sulfuric acid and water (NMB=−25%. Simulated CN concentrations in the continental BL were also biased low (NMB=−74% unless the number emission of anthropogenic primary particles was increased or a mechanism that results in particle formation in the BL was included. We ran a number of simulations where we included an empirical BL nucleation mechanism either using the activation-type mechanism (nucleation rate, J, proportional to gas-phase sulfuric acid concentration to the power one or kinetic-type mechanism (J proportional to sulfuric acid to the power two with a range of nucleation coefficients. We found that the seasonal CN cycle observed at continental BL sites was better simulated by BL particle formation (R²=0.3 than by increasing the number emission from primary anthropogenic sources (R²=0.18. The nucleation constants that resulted in best overall match between model and observed CN concentrations were

Effects of aromatics, olefins and distillation temperatures (T50 & T90) on particle mass and number emissions from gasoline direct injection (GDI) vehicles

International Nuclear Information System (INIS)

Zhu, Rencheng; Hu, Jingnan; Bao, Xiaofeng; He, Liqiang; Zu, Lei

2017-01-01

Abstratct: Fuel quality is among the primary reasons for severe vehicle pollution. A limited understanding of the effects of gasoline properties on modern vehicle emissions is one obstacle for the establishment of stricter fuel standards in China. The goal of this study was to evaluate the effects of aromatic and olefin contents and T50 and T90 (defined as the 50%v and 90%v distillation temperatures) on tailpipe emissions from gasoline direct injection (GDI) vehicles compliant with China 4 standards. Both gaseous and particle emissions using different types of gasoline were measured. Changing aromatic and olefin contents had relatively small impacts on fuel consumption. Compared with olefins and T90, the regulated gaseous emissions were impacted more by aromatics and T50. Evident decreases of the particle mass (PM) and particle number (PN) emissions were noticed when the aromatic content and T90 decreased. Reducing the olefin content slightly decreased the PM emissions and increased the PN emissions. With decreasing T50, the PM emissions increased and the PN emissions slightly decreased. These results suggest that aromatic content and T90 should be decreased to reduce particle emissions from GDI vehicles. The information presented in this study provides some suggestions for how to improve gasoline quality in China. - Highlights: • Effect of aromatics, olefins, T50 and T90 on GDI vehicle emissions was investigated. • Aromatics and olefins had little impact on fuel consumption and CO 2 emissions. • Reducing the aromatic content and T90 significantly decreased PM and PN emissions. • Changing the olefin content and T50 had a minor impact on particle emissions. • Thresholds of aromatics and T90 should be tightened in future gasoline regulations.

Particles and nuclei, letters

International Nuclear Information System (INIS)

2002-01-01

The present collection of letters from JINR, Dubna, contains eight separate records on the role of the complanar emission of particles in nuclear interaction for E 0 >10 16 eV detected in the stratosphere, 10 B nucleus fragment yields, nuclear teleportation (proposal for an experiment), invisible 'glue' bosons in model field theory, calculation of the ionization differential effective cross sections in fast ion-atom collisions, interactions of ultracold neutrons near surface of solids, g factors as a probe for high-spin structure of neutron-rich Dy isotopes, search for periodicities in experimental data by the autoregressive model methods

Studies on fast wave current drive in the JAERI tokamaks

International Nuclear Information System (INIS)

Kimura, H.; Yamamoto, T.; Fujii, T.; Kawashima, H.; Tamai, H.; Saigusa, M.; Imai, T.; Hamamatsu, K.; Fukuyama, A.

1991-01-01

Fast wave electron heating experiment (FWEH) on JFT-2M and JT-60 and analysis of fast wave current drive (FWCD) ability on JT-60U are presented. In the JFT-2M, absorption of fast waves have been investigated by using a phased four-loop antenna array. The absorption of the fast waves has been studied for various plasma parameters by using combination of other additional heating methods such as electron cyclotron heating (ECH) and ion cyclotron heating. It is shown that the absorption efficiency estimated from various methods well correlates with one calculated theoretically in single pass damping. Interaction of the fast waves with fast electrons in combination with ECH has been examined through the measurement of non-thermal electron cyclotron emission (ECE). The observed ECE during FWEH is well explained by the theoretical model, which indicates generation of the appreciable energetic fast electrons by the fast waves. New four-loop array antennas have been employed to improve the absorption of unidirectionally-propagating waves. Characteristics of antenna loading resistance can be reproduced by a coupling calculation code. In JT-60, FWEH experiment in combination with lower hybrid current drive was performed. Power absorption efficiency of fast wave is substantially improved in combination with LHCD of relatively low power for both phasing modes. Bulk electron heating is observed with high-k // mode and coupling with fast electron is confirmed in hard X-ray emission with low-k // mode. The results are consistent with theoretical prediction based on 1.D full wave code. Synergetic effects between FWEH and LHCD are found. Coupling calculation indicates that eight-loop antenna is favourable for keeping high directivity in the required N // -range. Current drive efficiency is calculated with 1-D full wave code including trapped particle effects and higher harmonic ion cyclotron damping

Polydopamine Particle-Filled Shape-Memory Polyurethane Composites with Fast Near-Infrared Light Responsibility.

Science.gov (United States)

Yang, Li; Tong, Rui; Wang, Zhanhua; Xia, Hesheng

2018-03-25

A new kind of fast near-infrared (NIR) light-responsive shape-memory polymer composites was prepared by introducing polydopamine particles (PDAPs) into commercial shape-memory polyurethane (SMPU). The toughness and strength of the polydopamine-particle-filled polyurethane composites (SMPU-PDAPs) were significantly enhanced with the addition of PDAPs due to the strong interface interaction between PDAPs and polyurethane segments. Owing to the outstanding photothermal effect of PDAPs, the composites exhibit a rapid light-responsive shape-memory process in 60 s with a PDAPs content of 0.01 wt%. Due to the excellent dispersion and convenient preparation method, PDAPs have great potential to be used as high-efficiency and environmentally friendly fillers to obtain novel photoactive functional polymer composites. © 2018 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Numerical study of the particle transport in fast neutron detectors with conversion layer

International Nuclear Information System (INIS)

Sedlackova, K.; Zatko, B.; Necas, V.

2012-01-01

This paper deals with fast neutron and recoil proton transport simulation using statistical analysis of Monte Carlo radiation transport code (MCNPX). Its possibilities in the detector design and optimization are presented. MCNPX proved as a very advantageous self-contained simulation program for fast neutron and secondary proton tracking. Simulations of respective particle transport through conversion layer of HDPE and further in the active volume of detector let us to follow important characteristics as neutron/proton flux density, reaction rate of elastic scattering on hydrogen nuclei and deposited energy as well as their dependencies on incident neutron energy and conversion layer/active region thickness. The efficiency of neutrons to protons conversion has been calculated and its maximum was reached for 500 μm thick conversion layer. The minimum active region thickness has been estimated to be about 300 μm.(authors)

Fast identification of the conduction-type of nanomaterials by field emission technique.

Science.gov (United States)

Yang, Xun; Gan, Haibo; Tian, Yan; Peng, Luxi; Xu, Ningsheng; Chen, Jun; Chen, Huanjun; Deng, Shaozhi; Liang, Shi-Dong; Liu, Fei

2017-10-12

There are more or less dopants or defects existing in nanomaterials, so they usually have different conduct-types even for the same substrate. Therefore, fast identification of the conduction-type of nanomaterials is very essential for their practical application in functional nanodevices. Here we use the field emission (FE) technique to research nanomaterials and establish a generalized Schottky-Nordheim (SN) model, in which an important parameter λ (the image potential factor) is first introduced to describe the effective image potential. By regarding λ as the criterion, their energy-band structure can be identified: (a) λ = 1: metal; (b) 0.5 p-type semiconductor. Moreover, this method can be utilized to qualitatively evaluate the doping-degree for a given semiconductor. We test numerically and experimentally a group of nanomaterial emitters and all results agree with our theoretical results very well, which suggests that our method based on FE measurements should be an ideal and powerful tool to fast ascertain the conduction-type of nanomaterials.

Light charged particle production in fast neutron-induced reactions on carbon (En=40 to 75 MeV) (II). Tritons and alpha particles

International Nuclear Information System (INIS)

Dufauquez, C.; Slypen, I.; Benck, S.; Meulders, J.P.; Corcalciuc, V.

2000-01-01

Double-differential cross sections for fast neutron-induced triton and alpha-particle production on carbon are reported at six incident neutron energies between 40 and 75 MeV. Angular distributions were measured at laboratory angles between 20 deg. and 160 deg. . Energy-differential, angle-differential and total cross sections are also reported. Experimental cross sections are compared to existing experimental data and to theoretical model calculations

Destabilization of Alfven eigenmodes by fast particles in W7-AS

International Nuclear Information System (INIS)

Zegenhagen, S.

2006-02-01

In the present thesis, a systematic study of beam driven Alfven eigenmodes in high-density and low-temperature plasmas of the W7-AS stellarator is performed. The goal of this thesis is twofold: (I) identification and description of fast particle driven Alfven instabilities in W7-AS, and (II) study of energetic particle losses induced by Alfven instabilities. A total of 133 different Alfven eigenmodes is studied in discharges from different experimental campaigns. The discharges are characterized by high density, n e =5 x 1019 m -3 to 2.5 x 1020 m -3 at relatively low temperatures of T e =T i =150..600 eV. Additional 13 events are found to have frequencies inside the EAE gap and could possibly be EAEs. Evidence for high-frequency Alfven eigenmodes (mirror- and helicity-induced Alfven eigenmodes) is seen, but can not be proven rigorously due to uncertain mode numbers and the complexity of the Alfven continuum. The remaining 41 Alfven eigenmodes can not be classified to be one of the above cases. (orig.)

Destabilization of Alfven eigenmodes by fast particles in W7-AS

Energy Technology Data Exchange (ETDEWEB)

Zegenhagen, S.

2006-02-15

In the present thesis, a systematic study of beam driven Alfven eigenmodes in high-density and low-temperature plasmas of the W7-AS stellarator is performed. The goal of this thesis is twofold: (I) identification and description of fast particle driven Alfven instabilities in W7-AS, and (II) study of energetic particle losses induced by Alfven instabilities. A total of 133 different Alfven eigenmodes is studied in discharges from different experimental campaigns. The discharges are characterized by high density, n{sub e}=5 x 1019 m{sup -3} to 2.5 x 1020 m{sup -3} at relatively low temperatures of T{sub e}=T{sub i}=150..600 eV. Additional 13 events are found to have frequencies inside the EAE gap and could possibly be EAEs. Evidence for high-frequency Alfven eigenmodes (mirror- and helicity-induced Alfven eigenmodes) is seen, but can not be proven rigorously due to uncertain mode numbers and the complexity of the Alfven continuum. The remaining 41 Alfven eigenmodes can not be classified to be one of the above cases. (orig.)

Particle acceleration during merging-compression plasma start-up in the Mega Amp Spherical Tokamak

Science.gov (United States)

McClements, K. G.; Allen, J. O.; Chapman, S. C.; Dendy, R. O.; Irvine, S. W. A.; Marshall, O.; Robb, D.; Turnyanskiy, M.; Vann, R. G. L.

2018-02-01

Magnetic reconnection occurred during merging-compression plasma start-up in the Mega Amp Spherical Tokamak (MAST), resulting in the prompt acceleration of substantial numbers of ions and electrons to highly suprathermal energies. Accelerated field-aligned ions (deuterons and protons) were detected using a neutral particle analyser at energies up to about 20 keV during merging in early MAST pulses, while nonthermal electrons have been detected indirectly in more recent pulses through microwave bursts. However no increase in soft x-ray emission was observed until later in the merging phase, by which time strong electron heating had been detected through Thomson scattering measurements. A test-particle code CUEBIT is used to model ion acceleration in the presence of an inductive toroidal electric field with a prescribed spatial profile and temporal evolution based on Hall-MHD simulations of the merging process. The simulations yield particle distributions with properties similar to those observed experimentally, including strong field alignment of the fast ions and the acceleration of protons to higher energies than deuterons. Particle-in-cell modelling of a plasma containing a dilute field-aligned suprathermal electron component suggests that at least some of the microwave bursts can be attributed to the anomalous Doppler instability driven by anisotropic fast electrons, which do not produce measurable enhancements in soft x-ray emission either because they are insufficiently energetic or because the nonthermal bremsstrahlung emissivity during this phase of the pulse is below the detection threshold. There is no evidence of runaway electron acceleration during merging, possibly due to the presence of three-dimensional field perturbations.

Quantitative comparisons of type 3 radio burst intensity and fast electron flux at 1 AU

Science.gov (United States)

Fitzenreiter, R. J.; Evans, L. G.; Lin, R. P.

1975-01-01

The flux of fast solar electrons and the intensity of the type 111 radio emission generated by these particles were compared at one AU. Two regimes were found in the generation of type 111 radiation: one where the radio intensity is linearly proportional to the electron flux, and another, which occurs above a threshold electron flux, where the radio intensity is approximately proportional to the 2.4 power of the electron flux. This threshold appears to reflect a transition to a different emission mechanism.

Quantitative comparisons of type 3 radio burst intensity and fast electron flux at 1 AU

International Nuclear Information System (INIS)

Fitzenreiter, R.J.; Evans, L.G.; Lin, R.P.

1975-09-01

The flux of fast solar electrons and the intensity of the type-III radio emission generated by these particles were compared at one AU. Two regimes were found in the generation of type-III radiation: one, where the radio intensity is linearly proportional to the electron flux, and another, which occurs above a threshold electron flux, where the radio intensity is approximately proportional to the 2.4 power of the electron flux. This threshold appears to reflect a transition to a different emission mechanism

Emission of high-energy charged particles at 00 in Ne-induced reactions

International Nuclear Information System (INIS)

Borcea, C.; Gierlik, E.; Kalinin, A.M.; Kalpakchieva, R.; Oganessia, Yu.Ts.; Pawlat, T.; Penionzhkevich, Yu.E.; Ryakhlyuk, A.V.

1982-01-01

Inclusive energy spectra have been measured for light charged particles emitted in the bombardment of 232 Th, 181 Ta, sup(nat)Ti and 12 C targets by 22 Ne ions at 178 MeV and sup(nat)Ti target by 20 Ne ions at 196 MeV. The reaction products were analysed and detected by means of a ΔE-E telescope placed in the focal plane of a magnetic spectrometer located at an angle of 0 deg with respect to the beam direction. In all the reactions studied light charged particles with an energy close to the respective calculated kinematic limit for a two-body exit channel are produced with relatively great probability. The results obtained make it possible to draw some conclusions about the reaction mechanism involving the emission of light charged particles

A Neuro-Fuzzy Multi Swarm FastSLAM Framework

OpenAIRE

Havangi, R.; Teshnehlab, M.; Nekoui, M. A.

2010-01-01

FastSLAM is a framework for simultaneous localization using a Rao-Blackwellized particle filter. In FastSLAM, particle filter is used for the mobile robot pose (position and orientation) estimation, and an Extended Kalman Filter (EKF) is used for the feature location's estimation. However, FastSLAM degenerates over time. This degeneracy is due to the fact that a particle set estimating the pose of the robot loses its diversity. One of the main reasons for loosing particle diversity in FastSLA...

Spontaneous photon emission from a non-relativistic free charged particle in collapse models: A case study

International Nuclear Information System (INIS)

Bassi, A.; Donadi, S.

2014-01-01

We study the photon emission rate of a non-relativistic charged particle interacting with an external classical noise through its position. Both the particle and the electromagnetic field are quantized. Under only the dipole approximation, the equations of motion can be solved exactly for a free particle, or a particle bounded by an harmonic potential. The physical quantity we will be interested in is the spectrum of the radiation emitted by the particle, due to the interaction with the noise. We will highlight several properties of the spectrum and clarify some issues appearing in the literature, regarding the exact mathematical formula of a spectrum for a free particle.

An optimised set-up for total reflection particle induced X-ray emission

International Nuclear Information System (INIS)

Kan, J.A. van; Vis, R.D.

1997-01-01

MeV proton beams at small angles of incidence (0-35 mrad) are used to analyse trace elements on flat surfaces such as Si wafers or quartz substrates. In these experiments, the particle induced X-ray emission (PIXE) signal is used in a new optimized set-up. This set-up is constructed in such a way that the X-ray detector can reach very large solid angles, larger than 1 sr. Use of these large detector solid angles, combined with the reduction of bremsstrahlung background, affords limits of detection (LOD) of the order of 10 10 at cm -2 using total reflection particle induced X-ray emission (TPIXE). The LODs from earlier TPIXE measurements in a non-optimized set-up are used to estimate LODs in the new TPIXE set-up. Si wafers with low surface concentrations of V, Ni, Cu and Ag are used as standards to calibrate the LODs found with this set-up. The metal concentrations are determined by total reflection X-ray fluorescence (TXRF). The TPIXE measurements are compared with TXRF measurements on the same wafers. (Author)

Monte Carlo problem and parallel computers, and how to do a fast particle mover on the STAR 100

International Nuclear Information System (INIS)

Sinz, K.H.P.H.

1975-01-01

Particle simulation problems of the Monte Carlo type are widely believed to be intrinsically highly scalar problems. In the absence of a definitive mathematical theorem to the contrary, this belief is based on the very apparent programming difficulties encountered on a vector machine. This class of problem is therefore thought to be ill-suited to highly parallel and vectorized computers. However, it is demonstrated by several examples that a particle mover is fully vectorizable. In the case of the CDC STAR 100 it is found that the performance of such a particle mover is not hopeless but hopeful, and is in fact helpful. One of the several possible vectorizations is estimated to yield a gain of a factor of 15 on the STAR over good serial coding on the same machine. This falls far short of the STAR's peak vector performance of 30 to 70 times scalar rates because certain fast vector instructions are not available and have to be simulated. The current STAR algorithm outperforms the carefully handcoded 7600 by a factor of 3. This performance margin is achievable despite the 7600's fivefold superior scalar capability. A more generally vectorized particle mover will always substantially outperform scalar coding on any machine equipped with a properly chosen set of fast vector instructions. (U.S.)

Simulating emission and chemical evolution of coarse sea-salt particles in the Community Multiscale Air Quality (CMAQ model

Directory of Open Access Journals (Sweden)

J. T. Kelly

2010-04-01

Full Text Available Chemical processing of sea-salt particles in coastal environments significantly impacts concentrations of particle components and gas-phase species and has implications for human exposure to particulate matter and nitrogen deposition to sensitive ecosystems. Emission of sea-salt particles from the coastal surf zone is known to be elevated compared to that from the open ocean. Despite the importance of sea-salt emissions and chemical processing, the US EPA's Community Multiscale Air Quality (CMAQ model has traditionally treated coarse sea-salt particles as chemically inert and has not accounted for enhanced surf-zone emissions. In this article, updates to CMAQ are described that enhance sea-salt emissions from the coastal surf zone and allow dynamic transfer of HNO₃, H₂SO₄, HCl, and NH₃ between coarse particles and the gas phase. Predictions of updated CMAQ models and the previous release version, CMAQv4.6, are evaluated using observations from three coastal sites during the Bay Regional Atmospheric Chemistry Experiment (BRACE in Tampa, FL in May 2002. Model updates improve predictions of NO₃⁻, SO₄²⁻, NH₄⁺, Na⁺, and Cl⁻ concentrations at these sites with only a 8% increase in run time. In particular, the chemically interactive coarse particle mode dramatically improves predictions of nitrate concentration and size distributions as well as the fraction of total nitrate in the particle phase. Also, the surf-zone emission parameterization improves predictions of total sodium and chloride concentration. Results of a separate study indicate that the model updates reduce the mean absolute error of nitrate predictions at coastal CASTNET and SEARCH sites in the eastern US. Although the new model features improve performance relative to CMAQv4.6, some persistent differences exist between observations and predictions

Coal emissions adverse human health effects associated with ultrafine/nano-particles role and resultant engineering controls.

Science.gov (United States)

Oliveira, Marcos L S; Navarro, Orlando G; Crissien, Tito J; Tutikian, Bernardo F; da Boit, Kátia; Teixeira, Elba C; Cabello, Juan J; Agudelo-Castañeda, Dayana M; Silva, Luis F O

2017-10-01

There are multiple elements which enable coal geochemistry: (1) boiler and pollution control system design parameters, (2) temperature of flue gas at collection point, (3) feed coal and also other fuels like petroleum coke, tires and biomass geochemistry and (4) fuel feed particle size distribution homogeneity distribution, maintenance of pulverisers, etc. Even though there is a large number of hazardous element pollutants in the coal-processing industry, investigations on micrometer and nanometer-sized particles including their aqueous colloids formation reactions and their behaviour entering the environment are relatively few in numbers. X-ray diffraction (XRD), High Resolution-Transmission Electron microscopy (HR-TEM)/ (Energy Dispersive Spectroscopy) EDS/ (selected-area diffraction pattern) SAED, Field Emission-Scanning Electron Microscopy (FE-SEM)/EDS and granulometric distribution analysis were used as an integrated characterization techniques tool box to determine both geochemistry and nanomineralogy for coal fly ashes (CFAs) from Brazil´s largest coal power plant. Ultrafine/nano-particles size distribution from coal combustion emissions was estimated during the tests. In addition the iron and silicon content was determined as 54.6% of the total 390 different particles observed by electron bean, results aimed that these two particles represent major minerals in the environment particles normally. These data may help in future investigations to asses human health actions related with nano-particles. Copyright © 2017 Elsevier Inc. All rights reserved.

Battery condenser system particulate emission factors for cotton gins: Particle size distribution characteristics

Science.gov (United States)

This report is part of a project to characterize cotton gin emissions from the standpoint of total particulate stack sampling and particle size analyses. In 2013, the Environmental Protection Agency (EPA) published a more stringent standard for particulate matter with nominal diameter less than or e...

Light particle and gamma ray emission measurements in heavy-ion reactions. Progress report

International Nuclear Information System (INIS)

Petitt, G.A.

1982-01-01

The development of a position-sensitive neutron detector and a data acquisition system at HHIRF for studying light particle emission in heavy ion reactions is described. Results are presented and discussed for the reactions 12 C + 158 Gd, 13 C + 157 Gd, and 20 Ne + 150 Nd

Use of GSR particle analysis program on an analytical SEM to identify sources of emission of airborne particles

International Nuclear Information System (INIS)

Chan, Y.C.; Trumper, J.; Bostrom, T.

2002-01-01

Full text: High concentrations of airborne particles, in particular PM 10 (particulate matter 10 , but has been little used in Australia for airborne particulates. Two sets of 15 mm PM 10 samples were collected in March and April 2000 from two sites in Brisbane, one within a suburb and one next to an arterial road. The particles were collected directly onto double-sided carbon tapes with a cascade impactor attached to a high-volume PM 10 sampler. The carbon tapes were analysed in a JEOL 840 SEM equipped with a Be-window energy-dispersive X-ray detector and Moran Scientific microanalysis system. An automated Gun Shot Residue (GSR) program was used together with backscattered electron imaging to characterise and analyse individual particulates. About 6,000 particles in total were analysed for each set of impactor samples. Due to limitations of useful pixel size, only particles larger than about 0.5 μm could be analysed. The size, shape and estimated elemental composition (from Na to Pb) of the particles were subjected to non-hierarchical cluster analysis and the characteristics of the clusters were related to their possible sources of emission. Both samples resulted in similar particle clusters. The particles could be classified into three main categories non-spherical (58% of the total number of analysed particles, shape factor >1 1), spherical (15%) and 'carbonaceous' (27%, ie with unexplained % of elemental mass >75%). Non-spherical particles were mainly sea salt and soil particles, and a small amount of iron, lead and mineral dust. The spherical particles were mainly sea salt particles and flyash, and a small amount of iron, lead and secondary sulphate dust. The carbonaceous particles included carbon material mixed with secondary aerosols, roadside dust, sea salt or industrial dust. The arterial road sample also contained more roadside dust and less secondary aerosols than the suburb sample. Current limitations with this method are the minimum particle size

CIRCUMSOLAR ENERGETIC PARTICLE DISTRIBUTION ON 2011 NOVEMBER 3

Energy Technology Data Exchange (ETDEWEB)

Gómez-Herrero, R.; Blanco, J.J.; Rodríguez-Pacheco, J. [SRG, Universidad de Alcalá, E-28871 Alcalá de Henares (Spain); Dresing, N.; Klassen, A.; Heber, B.; Banjac, S. [IEAP, Christian-Albrechts-Universität zu Kiel, D-24118 Kiel (Germany); Lario, D. [The Johns Hopkins University, Applied Physics Laboratory, Laurel, MD 20723 (United States); Agueda, N. [Departament d' Astronomia i Meteorologia. Institut de Ciències del Cosmos. Universitat de Barcelona, E-08028 Barcelona (Spain); Malandraki, O. E., E-mail: raul.gomezh@uah.es [IAASARS, National Observatory of Athens, GR-15236 Penteli (Greece)

2015-01-20

Late on 2011 November 3, STEREO-A, STEREO-B, MESSENGER, and near-Earth spacecraft observed an energetic particle flux enhancement. Based on the analysis of in situ plasma and particle observations, their correlation with remote sensing observations, and an interplanetary transport model, we conclude that the particle increases observed at multiple locations had a common single-source active region and the energetic particles filled a very broad region around the Sun. The active region was located at the solar backside (as seen from Earth) and was the source of a large flare, a fast and wide coronal mass ejection, and an EIT wave, accompanied by type II and type III radio emission. In contrast to previous solar energetic particle events showing broad longitudinal spread, this event showed clear particle anisotropies at three widely separated observation points at 1 AU, suggesting direct particle injection close to the magnetic footpoint of each spacecraft, lasting for several hours. We discuss these observations and the possible scenarios explaining the extremely broad particle spread for this event.

Morphology and Optical Properties of Black-Carbon Particles Relevant to Engine Emissions

Science.gov (United States)

Michelsen, H. A.; Bambha, R.; Dansson, M. A.; Schrader, P. E.

2013-12-01

Black-carbon particles are believed to have a large influence on climate through direct radiative forcing, reduction of surface albedo of snow and ice in the cryosphere, and interaction with clouds. The optical properties and morphology of atmospheric particles containing black carbon are uncertain, and characterization of black carbon resulting from engines emissions is needed. Refractory black-carbon particles found in the atmosphere are often coated with unburned fuel, sulfuric acid, water, ash, and other combustion by-products and atmospheric constituents. Coatings can alter the optical and physical properties of the particles and therefore change their optical properties and cloud interactions. Details of particle morphology and coating state can also have important effects on the interpretation of optical diagnostics. A more complete understanding of how coatings affect extinction, absorption, and incandescence measurements is needed before these techniques can be applied reliably to a wide range of particles. We have investigated the effects of coatings on the optical and physical properties of combustion-generated black-carbon particles using a range of standard particle diagnostics, extinction, and time-resolved laser-induced incandescence (LII) measurements. Particles were generated in a co-flow diffusion flame, extracted, cooled, and coated with oleic acid. The diffusion flame produces highly dendritic soot aggregates with similar properties to those produced in diesel engines, diffusion flames, and most natural combustion processes. A thermodenuder was used to remove the coating. A scanning mobility particle sizer (SMPS) was used to monitor aggregate sizes; a centrifugal particle mass analyzer (CPMA) was used to measure coating mass fractions, and transmission electron microscopy (TEM) was used to characterize particle morphologies. The results demonstrate important differences in optical measurements between coated and uncoated particles.

Theoretical model of Orion gamma emission: acceleration, propagation and interaction of energetic particles in the interstellar medium

International Nuclear Information System (INIS)

Parizot, Etienne

1997-01-01

This research thesis reports the development of a general model for the study of the propagation and interaction of energetic particles (cosmic rays, and so on) in the interstellar medium (ISM). The first part addresses the development of theoretical and numerical tools. The author presents cosmic rays and energetic particles, presents and describes the various processes related to high-energy particles (matter ionisation, synchrotron and Bremsstrahlung radiation, Compton scattering, nuclear processes), addresses the transport and acceleration of energetic particles (plasmas, magnetic fields and energetic particles, elements of kinetic theory, transport and acceleration of energetic particles), and describes the general model of production of γ nuclear lines and of secondary nuclei. The second part addresses the gamma signature of a massive star in a dense medium: presentation and description of massive stars and of the circumstellar medium, life, death and gamma resurrection of a massive star at the heart of a cloud. The third part addresses the case of the gamma emission by Orion, and more particularly presents a theoretical model of this emission. Some generalities and perspectives (theoretical as well as observational) are then stated [fr

A study of complex particle emission in the pre-equilibrium statistical model

International Nuclear Information System (INIS)

Miao Rongzhi; Wu Guohua

1986-01-01

A concept of the quasi-composite system in the process of the pre-equilibrium emission is presented in this paper. On the basis of the principle of detailed balance, the existence of the factor, [γ β ω(π β , 0, ν β , 0, E-U)g π,ν ], has been proved with an account of the distinguishabllity between protons and neutrons. A formula for the rate of the complex particle emission in the pre-equilibrium process can be obtained. The theoretical calculation results fit the experimental data quite well, especially in the high energy part of the energy spectrum the agreement are much better than ever before

Ultra fast atomic process in X-ray emission by inner-shell ionization

Energy Technology Data Exchange (ETDEWEB)

Moribayashi, Kengo; Sasaki, Akira [Japan Atomic Energy Research Inst., Neyagawa, Osaka (Japan). Kansai Research Establishment; Tajima, T

1998-03-01

An ultra-fast atomic process together with X-ray emission by inner-shell ionization using high intensity (10{sup 18} W/cm{sup 2}) short pulse (20fs) X-ray is studied. A new class of experiment is proposed and a useful pumping source is suggested. In this method, it is found that the gain value of X-ray laser amounts to larger than 1000(1/cm) with use of the density of 10{sup 22}/cm{sup 3} of carbon atom. Electron impact ionization effect and initial density effect as well as intensity of pumping source effect are also discussed. (author)

Quantitative comparisons of type III radio burst intensity and fast electron flux at 1 AU

Science.gov (United States)

Fitzenreiter, R. J.; Evans, L. G.; Lin, R. P.

1976-01-01

We compare the flux of fast solar electrons and the intensity of the type III radio emission generated by these particles at 1 AU. We find that there are two regimes in the generation of type III radiation: one where the radio intensity is linearly proportional to the electron flux, and the second regime, which occurs above a threshold electron flux, where the radio intensity is proportional to the approximately 2.4 power of the electron flux. This threshold appears to reflect a transition to a different emission mechanism.

Fast and reliable method for computing free-bound emission coefficients for hydrogenic ions

Energy Technology Data Exchange (ETDEWEB)

Sarmiento, A; Canto, J

1985-12-01

An approximate formula for the computation of the free-bound emission coefficient for hydrogenic ions is presented. The approximation is obtained through a manipulation of the (free-bound) Gaunt factor which intentionally distinguish the dependence on frequency from the dependence on temperature and ionic composition. Numerical tests indicate that the derived formula is very precise, fast and easy to use, making the calculation of the free-bound contribution from an ionized region of varying temperature and ionic composition a very simple and time-saving task.

Fast neutrons: Inexpensive and reliable tool to investigate high-LET particle radiobiology

International Nuclear Information System (INIS)

Gueulette, J.; Slabbert, J.P.; Bischoff, P.; Denis, J.M.; Wambersie, A.; Jones, D.

2010-01-01

Radiation therapy with carbon ions as well as missions into outer space have boosted the interest for high-LET particle radiobiology. Optimization of treatments in accordance with technical developments, as well as the radioprotection of cosmonauts during long missions require that research in these domains continue. Therefore suitable radiation fields are needed. Fast neutrons and carbon ions exhibit comparable LET values and similar radiobiological properties. Consequently, the findings obtained with each radiation quality could be shared to benefit knowledge in all concerned domains. The p(66+Be) neutron therapy facilities of iThemba LABS (South Africa) and the p(65)+Be neutron facility of Louvain-la-Neuve (Belgium) are in constant use to do radiobiological research for clinical applications with fast neutrons. These beams - which comply with all physical and technical requirements for clinical applications - are now fully reliable, easy to use and frequently accessible for radiobiological investigations. These facilities thus provide unique opportunities to undertake radiobiological experimentation, especially for investigations that require long irradiation times and/or fractionated treatments.

In-situ measurements of ice nucleating particles with FINCH (Fast Ice Nucleus Chamber)

Science.gov (United States)

Kohl, Rebecca; Frank, Fabian; Curtius, Joachim; Rose, Diana

2017-04-01

Ice nucleating particles (INPs), which are a small fraction of the total aerosol population, are capable of triggering ice formation under atmospheric conditions. Since INPs play an important role for the radiative properties of clouds as well as for the formation of precipitation it is important to get quantitative information on the ice activity of various atmospheric aerosol species. With the Fast Ice Nucleus Chamber (FINCH; Bundke et al., 2008) the number concentration of INP is determined at different freezing temperatures and supersaturations. In contrast to other commonly used INP counters, i.e., continuous flow diffusion chambers (CFDCs, DeMott et al., 2011), in FINCH the supersaturation is reached by mixing the sample flow of ambient aerosol with a warm moist as well as a cold dry airflow. By changing the flow rates and temperatures of the individual airflows the freezing temperature (down to -50°C) and supersaturation (up to above water saturation) can be varied relatively quickly. Particles that are ice active at the prescribed freezing temperature and supersaturation grow to crystals and are counted by a home-built optical particle counter (OPC) mounted below the chamber (Bundke et al., 2010). FINCH was operated during the four-week INUIT-BACCHUS-ACTRIS field campaign in Cyprus in April 2016. The measuring site was the location of the Cyprus Atmospheric Observatory (CAO) at Agia Marina Xyliatou, which is typically influenced by dust from the Sahara and the Middle East, an aerosol that is known to have relatively good ice nucleating ability. First results from this campaign will be presented. Acknowledgements: The authors thank the entire INUIT-BACCHUS-ACTRIS campaign team for their cooperation and support. The INUIT-2 project is financed by the German Research Foundation DFG (FOR 1525). The INUIT-Cyprus campaign is a cooperation with the EU-funded project BACCHUS and is also funded by ACTRIS-TNA. References: Bundke, U., Nillius, B., Jaenicke, R

PAH, BTEX, carbonyl compound, black-carbon, NO2 and ultrafine particle dynamometer bench emissions for Euro 4 and Euro 5 diesel and gasoline passenger cars

Science.gov (United States)

Louis, Cédric; Liu, Yao; Tassel, Patrick; Perret, Pascal; Chaumond, Agnès; André, Michel

2016-09-01

Although implementing Diesel particulate filters (DPF) and other novel aftertreatment technologies makes it possible to achieve significant reductions in particle mass emissions, it may induce the release of ultrafine particles and emissions of many other unregulated compounds. This paper focuses on (i) ultrafine particles, black carbon, BTEX, PAH, carbonyl compounds, and NO2 emissions from Euro 4 and Euro 5 Diesel and gasoline passenger cars, (ii) the influence of driving conditions (e.g., cold start, urban, rural and motorway conditions), and (iii) the impact of additive and catalysed DPF devices on vehicle emissions. Chassis dynamometer tests were conducted on four Euro 5 vehicles and two Euro 4 vehicles: gasoline vehicles with and without direct injection system and Diesel vehicles equipped with additive and catalysed particulate filters. The results showed that compared to hot-start cycles, cold-start urban cycles increased all pollutant emissions by a factor of two. The sole exception was NO2, which was reduced by a factor of 1.3-6. Particulate and black carbon emissions from the gasoline engines were significantly higher than those from the Diesel engines equipped with DPF. Moreover, the catalysed DPF emitted about 3-10 times more carbonyl compounds and particles than additive DPF, respectively, during urban driving cycles, while the additive DPF vehicles emitted 2 and 5 times more BTEX and carbonyl compounds during motorway driving cycles. Regarding particle number distribution, the motorway driving cycle induced the emission of particles smaller in diameter (mode at 15 nm) than the urban cold-start cycle (mode at 80-100 nm). The results showed a clear positive correlation between particle, black carbon, and BTEX emissions, and a negative correlation between particles and NO2.

Population of vibrational levels of carbon dioxide by cylindrical fast ionization wave

KAUST Repository

Levko, Dmitry

2017-09-08

The population of vibrational levels of carbon dioxide (CO2) by a cylindrical fast ionization wave is analyzed using a one-dimensional Particle-in-Cell Monte Carlo collisions model. The model takes into account the inelastic electron-neutral collisions as well as the super-elastic collisions between electrons and excited species. We observe an efficient population of only the first two levels of the symmetric and asymmetric vibrational modes of CO2 by means of a fast ionization wave. The excitation of other higher vibrational modes by the fast ionization wave is inefficient. Additionally, we observe a strong influence of the secondary electron emission on the population of vibrational states of CO2. This effect is associated with the kinetics of high energy electrons generated in the cathode sheath.

African Anthropogenic Combustion Emissions: Estimate of Regional Mortality Attributable to Fine Particle Concentrations in 2030

Science.gov (United States)

Liousse, C.; Roblou, L.; Assamoi, E.; Criqui, P.; Galy-Lacaux, C.; Rosset, R.

2014-12-01

Fossil fuel (traffic, industries) and biofuel (domestic fires) emissions of gases and particles in Africa are expected to significantly increase in the near future, particularly due to rapid growth of African cities and megacities. In this study, we will present the most recent developments of African combustion emission inventories, including African specificities. Indeed, a regional fossil fuel and biofuel inventory for gases and particulates described in Liousse et al. (2014) has been developed for Africa at a resolution of 0.25° x 0.25° for the years 2005 and 2030. For 2005, the original database of Junker and Liousse (2008) was used after modification for updated regional fuel consumption and emission factors. Two prospective inventories for 2030 are derived based on Prospective Outlook on Long-term Energy Systems (POLES) model (Criqui, 2001). The first is a reference scenario (2030ref) with no emission controls and the second is for a "clean" scenario (2030ccc*) including Kyoto policy and African specific emission control. This inventory predicts very large increases of pollutant emissions in 2030 (e.g. contributing to 50% of global anthropogenic organic particles), if no emission regulations are implemented. These inventories have been introduced in RegCM4 model. In this paper we will focus on aerosol modelled concentrations in 2005, 2030ref and 2030ccc*. Spatial distribution of aerosol concentrations will be presented with a zoom at a few urban and rural sites. Finally mortality rates (respiratory, cardiovascular) caused by anthropogenic PM2.5 increase from 2005 to 2030, calculated following Lelieveld et al. (2013), will be shown for each scenarios. To conclude, this paper will discuss the effectiveness of scenarios to reduce emissions, aerosol concentrations and mortality rates, underlining the need for further measurements scheduled in the frame of the new DACCIWA (Dynamics-Aerosol-Chemistry-Cloud Interactions) program.

Particle Acceleration, Magnetic Field Generation and Emission from Relativistic Jets

Science.gov (United States)

Nishikawa, K.-I.; Hardee, P.; Hededal, C.; Mizuno, Yosuke; Fishman, G. Jerry; Hartmann, D. H.

2006-01-01

Nonthermal radiation observed from astrophysical systems containing relativistic jets and shocks, e.g., active galactic nuclei (AGNs), gamma-ray bursts (GRBs), supernova remnants, and Galactic microquasar systems usually have power-law emission spectra. Fermi acceleration is the mechanism usually assumed for the acceleration of particles in astrophysical environments. Recent PIC simulations using injected relativistic electron-ion (electro-positron) jets show that particle acceleration occurs within the downstream jet, rather than by the scattering of particles back and forth across the shock as in Fermi acceleration. Shock acceleration' is a ubiquitous phenomenon in astrophysical plasmas. Plasma waves and their associated instabilities (e.g., the Buneman instability, other two-streaming instability, and the Weibel instability) created in the shocks are responsible for particle (electron, positron, and ion) acceleration. The simulation results show that the Weibel instability is responsible for generating and amplifying highly nonuniform, small-scale magnetic fields. These magnetic fields contribute to the electron's transverse deflection behind the jet head. The "jitter" radiation from deflected electrons has different spectral properties than synchrotron radiation which is calculated in a uniform magnetic field. This jitter radiation may be important to understanding the complex time evolution and/or spectral structure in gamma-ray bursts, relativistic jets, and supernova remnants. We will review recent PIC simulations of relativistic jets and try to make a connection with observations.

Correction of Doppler broadening of {gamma}-ray lines induced by particle emission in heavy-ion induced fusion-evaporation reactions

Energy Technology Data Exchange (ETDEWEB)

Nyberg, J; Seweryniak, D; Fahlander, C; Insua-Cao, P [Uppsala Univ. (Sweden). Dept. of Radiation Sciences; Johnson, A; Cederwall, B [Manne Siegbahn Inst. of Physics, Stockholm (Sweden); [Royal Inst. of Tech., Stockholm (Sweden); Adamides, E; Piiparinen, M [National Centre for Scientific Research, Ag. Paraskevi, Attiki (Greece); Atac, A; Norlin, L O [Niels Bohr Inst., Copenhagen (Denmark); Ideguchi, E; Mitarai, S [Kyushu Univ., Fukuoka (Japan). Dept. of Physics; Julin, R; Juutinen, S; Tormanen, S; Virtanen, A [Jyvaeskylae Univ. (Finland). Dept. of Physics; Karczmarczyk, W; Kownacki, J [Warsaw Univ. (Poland); Schubart, R [Hahn-Meitner-Institut Berlin GmbH (Germany)

1992-08-01

The effect of particle emission on the peak shape of {gamma}-ray lines have been investigated using the NORDBALL detector system. By detecting neutrons, protons and {alpha} particles emitted in the {sup 32}S (95 MeV) + {sup 27}Al reaction, the energy and direction of emission of the residual nuclei could be determined and subsequently used for an event-by -event Doppler correction of the detected {gamma} rays. Extensive Monte Carlo simulations were performed to study how the different Doppler phenomena influence the peak shape and in particular which particle detector properties are important for the Doppler correction. (author). 2 refs., 1 tab., 4 figs.

Traffic generated non-exhaust particulate emissions from concrete pavement: A mass and particle size study for two-wheelers and small cars

Science.gov (United States)

Aatmeeyata; Kaul, D. S.; Sharma, Mukesh

This study aimed to understand the non-exhaust (NE) emission of particles from wear of summer tire and concrete pavement, especially for two wheelers and small cars. A fully enclosed laboratory-scale model was fabricated to simulate road tire interaction with a facility to collect particles in different sizes. A road was cast using the M-45 concrete mixture and the centrifugal casting method. It was observed that emission of large particle non exhaust emission (LPNE) as well as PM 10 and PM 2.5 increased with increasing load. The LPNE was 3.5 mg tire -1 km -1 for a two wheeler and 6.4 mg tire -1 km -1 for a small car. The LPNE can lead to water pollution through water run-off from the roads. The contribution of the PM 10 and PM 2.5 was smaller compared to the LPNE particles (less than 0.1%). About 32 percent of particle mass of PM 10 was present below 1 μm. The number as well as mass size distribution for PM 10 was observed to be bi-modal with peaks at 0.3 μm and 4-5 μm. The NE emissions did not show any significant trend with change in tire pressure.

Detection of special nuclear material from delayed neutron emission induced by a dual-particle monoenergetic source

Energy Technology Data Exchange (ETDEWEB)

Mayer, M. [Department of Mechanical and Nuclear Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802 (United States); Nattress, J.; Jovanovic, I., E-mail: ijov@umich.edu [Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, Michigan 48109 (United States)

2016-06-27

Detection of unique signatures of special nuclear materials is critical for their interdiction in a variety of nuclear security and nonproliferation scenarios. We report on the observation of delayed neutrons from fission of uranium induced in dual-particle active interrogation based on the {sup 11}B(d,n γ){sup 12}C nuclear reaction. Majority of the fissions are attributed to fast fission induced by the incident quasi-monoenergetic neutrons. A Li-doped glass–polymer composite scintillation neutron detector, which displays excellent neutron/γ discrimination at low energies, was used in the measurements, along with a recoil-based liquid scintillation detector. Time-dependent buildup and decay of delayed neutron emission from {sup 238}U were measured between the interrogating beam pulses and after the interrogating beam was turned off, respectively. Characteristic buildup and decay time profiles were compared to the common parametrization into six delayed neutron groups, finding a good agreement between the measurement and nuclear data. This method is promising for detecting fissile and fissionable materials in cargo scanning applications and can be readily integrated with transmission radiography using low-energy nuclear reaction sources.

Size-segregated emissions and metal content of vehicle-emitted particles as a function of mileage: Implications to population exposure

International Nuclear Information System (INIS)

Golokhvast, Kirill S.; Chernyshev, Valery V.; Chaika, Vladimir V.; Ugay, Sergey M.; Zelinskaya, Elena V.; Tsatsakis, Aristidis M.; Karakitsios, Spyros P.; Sarigiannis, Denis A.

2015-01-01

The study aims at investigating the characteristics (size distribution, active surface and metal content) of particles emitted by cars as a function of mileage using a novel methodology for characterizing particulate emissions captured by Exhaust Gas Suspension (EGS). EGS was obtained by passing the exhaust gases through a container of deionized water. EGS analysis was performed using laser granulometry, electron scanning microscopy, and high resolution mass spectrometry. Implications of the differences in key features of the emitted particles on population exposure were investigated using numerical simulation for estimating size-segregated PM deposition across human respiratory tract (HRT). It was found that vehicle mileage, age and the respective emissions class have almost no effect on the size distribution of the exhaust gas particulate released into the environment; about half of the examined vehicles with low mileage were found to release particles of aerodynamic diameter above 10 μm. The exhaust gas particulate detected in the EGS of all cars can be classified into three major size classes: (1) 0.1–5 µm – soot and ash particles, metals (Au, Pt, Pd, Ir); (2) 10–30 µm – metal (Cr, Fe, Cu, Zr, Ni) and ash particles; (3) 400–1,000 µm – metal (Fe, Cr, Pb) and ash particles. Newer vehicles with low mileage are substantial sources of soot and metal particles with median diameter of 200 nm with a higher surface area (up to 89,871.16 cm 2 /cm 3 ). These tend to deposit in the lower part of the human respiratory tract. - Highlights: • Car mileage has virtually no effect on the size of the solid particles released. • Newer diesel vehicles emit particles of lower aerodynamic diameter. • Particle active surface emitted by newer vehicles is on average 3 times higher. • Real-life emissions were translated into actual internal PM exposure.

Size-segregated emissions and metal content of vehicle-emitted particles as a function of mileage: Implications to population exposure

Energy Technology Data Exchange (ETDEWEB)

Golokhvast, Kirill S.; Chernyshev, Valery V.; Chaika, Vladimir V.; Ugay, Sergey M. [Far Eastern Federal University, Vladivostok (Russian Federation); Zelinskaya, Elena V. [National Research Irkutsk State Technical University, Irkutsk (Russian Federation); Tsatsakis, Aristidis M. [University of Crete, Medical School, Department of Toxicology and Forensic Science, Heraklion, Crete (Greece); Karakitsios, Spyros P. [Aristotle University of Thessaloniki, Department of Chemical Engineering, Thessaloniki (Greece); Sarigiannis, Denis A., E-mail: denis@eng.auth.gr [Aristotle University of Thessaloniki, Department of Chemical Engineering, Thessaloniki (Greece)

2015-10-15

The study aims at investigating the characteristics (size distribution, active surface and metal content) of particles emitted by cars as a function of mileage using a novel methodology for characterizing particulate emissions captured by Exhaust Gas Suspension (EGS). EGS was obtained by passing the exhaust gases through a container of deionized water. EGS analysis was performed using laser granulometry, electron scanning microscopy, and high resolution mass spectrometry. Implications of the differences in key features of the emitted particles on population exposure were investigated using numerical simulation for estimating size-segregated PM deposition across human respiratory tract (HRT). It was found that vehicle mileage, age and the respective emissions class have almost no effect on the size distribution of the exhaust gas particulate released into the environment; about half of the examined vehicles with low mileage were found to release particles of aerodynamic diameter above 10 μm. The exhaust gas particulate detected in the EGS of all cars can be classified into three major size classes: (1) 0.1–5 µm – soot and ash particles, metals (Au, Pt, Pd, Ir); (2) 10–30 µm – metal (Cr, Fe, Cu, Zr, Ni) and ash particles; (3) 400–1,000 µm – metal (Fe, Cr, Pb) and ash particles. Newer vehicles with low mileage are substantial sources of soot and metal particles with median diameter of 200 nm with a higher surface area (up to 89,871.16 cm{sup 2}/cm{sup 3}). These tend to deposit in the lower part of the human respiratory tract. - Highlights: • Car mileage has virtually no effect on the size of the solid particles released. • Newer diesel vehicles emit particles of lower aerodynamic diameter. • Particle active surface emitted by newer vehicles is on average 3 times higher. • Real-life emissions were translated into actual internal PM exposure.

Wood burning stoves and small boilers - particle emissions and reduction initiatives; Braendeovne og smae kedler - partikelemissioner og reduktionstiltag

Energy Technology Data Exchange (ETDEWEB)

Illerup, J B; Capral Henriksen, T; Lundhede, T [Danmarks Miljoeundersoegelser, Aarhus Universitet, Aarhus (Denmark); Breugel, C van; Zoellner Jensen, N [Miljoestyrelsen, Copenhagen (Denmark)

2007-06-15

Pollution from burning wood in private households, and the environmental and health consequences of this is determined in practice by a complicated interaction between a number of factors, including firing habits, fuel, type of stove/boiler, chimney and location of the chimney in relation to the surroundings. This report maps out the technologies used today for burning wood in private households, how these technologies contribute to particle emissions and which technologies may potentially reduce emissions of particles from burning wood in households in Denmark. Moreover, the possible emissions reductions and the financial costs incurred by consumers from different initiatives have been estimated. This report does not deal with possible initiatives for improvement of firing habits, fuel quality and chimneys. (au)

Fireplace and woodstove fine particle emissions from combustion of western Mediterranean wood types

Science.gov (United States)

Alves, Célia; Gonçalves, Cátia; Fernandes, Ana Patrícia; Tarelho, Luís; Pio, Casimiro

2011-08-01

Wood from seven species of trees grown in the Portuguese forest ( Pinus pinaster, Eucalyptus globulus, Quercus suber, Acacia longifolia, Quercus faginea, Olea europea and Quercus ilex rotundifolia), and briquettes produced from forest biomass waste were burned in a fireplace and in a woodstove to determine the chemical composition of fine particle (PM 2.5) emissions. Samples were analysed for organic and elemental carbon (OC/EC), water soluble ions (Na +, NH 4+, K +, Mg 2+, Ca 2+, Cl -, NO 3- and SO 42-) and 67 elements. The PM 2.5 emission factors (g kg - 1 fuel burned, dry basis) were in the ranges 9.9-20.2 and 4.2-16.3, respectively, for the fireplace and the woodstove. Organic carbon contributed to about 50% of the fine particle mass in the emissions from every wood species studied in both burning appliances. The carbonaceous component of PM 2.5 was dominated by organic carbon, accounting for more than 85% of the total carbon (TC): OC/TC ranged from 0.85 to 0.96 (avg. 0.92) for the fireplace and from 0.86 to 0.97 (avg. 0.93) for the woodstove. The water-soluble ions accounted for 0.64 to 11.3% of the PM 2.5 mass emitted from the fireplace, whereas mass fractions between 0.53 and 13.6% were obtained for the woodstove. The golden wattle wood smoke showed a much higher ionic content than the emissions from the other wood types. Trace elements represented 0.4 to 2.5% and 0.2 to 2.2% of the PM 2.5 mass emitted, respectively, from the fireplace and the woodstove, which corresponded to average total emissions of 132 ± 77.3 mg kg - 1 and 93.4 ± 60.8 mg kg - 1 of wood burned. Among these, K, Pb, Al, Mn and Sr were present in all samples. From the emission profiles of the individual experiments, composite wood combustion profiles are suggested with the aid of a cluster analysis.

Formation of secondary organic aerosol coating on black carbon particles near vehicular emissions

Science.gov (United States)

Lee, Alex K. Y.; Chen, Chia-Li; Liu, Jun; Price, Derek J.; Betha, Raghu; Russell, Lynn M.; Zhang, Xiaolu; Cappa, Christopher D.

2017-12-01

Black carbon (BC) emitted from incomplete combustion can result in significant impacts on air quality and climate. Understanding the mixing state of ambient BC and the chemical characteristics of its associated coatings is particularly important to evaluate BC fate and environmental impacts. In this study, we investigate the formation of organic coatings on BC particles in an urban environment (Fontana, California) under hot and dry conditions using a soot-particle aerosol mass spectrometer (SP-AMS). The SP-AMS was operated in a configuration that can exclusively detect refractory BC (rBC) particles and their coatings. Using the -log(NOx / NOy) ratio as a proxy for photochemical age of air masses, substantial formation of secondary organic aerosol (SOA) coatings on rBC particles was observed due to active photochemistry in the afternoon, whereas primary organic aerosol (POA) components were strongly associated with rBC from fresh vehicular emissions in the morning rush hours. There is also evidence that cooking-related organic aerosols were externally mixed from rBC. Positive matrix factorization and elemental analysis illustrate that most of the observed SOA coatings were freshly formed, providing an opportunity to examine SOA coating formation on rBCs near vehicular emissions. Approximately 7-20 wt % of secondary organic and inorganic species were estimated to be internally mixed with rBC on average, implying that rBC is unlikely the major condensation sink of SOA in this study. Comparison of our results to a co-located standard high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS) measurement suggests that at least a portion of SOA materials condensed on rBC surfaces were chemically different from oxygenated organic aerosol (OOA) particles that were externally mixed with rBC, although they could both be generated from local photochemistry.

Modified Sternglass theory for the emission of secondary electrons by fast-electron impact

International Nuclear Information System (INIS)

Suszcynsky, D.M.; Borovsky, J.E.

1992-01-01

The Sternglass theory [Sternglass, Phys. Rev. 108, 1 (1957)] for fast-ion-induced secondary-electron emission from metals has been modified to predict the secondary-electron yield from metals impacted by energetic (several keV to about 200 keV) electrons. The primary modification of the theory accounts for the contribution of the backscattered electrons to the production of secondary electrons based on a knowledge of the backscattered-electron energy distribution. The modified theory is in reasonable agreement with recent experimental data from gold targets in the 6--30-keV electron energy range

Emission from small dust particles in diffuse and molecular cloud medium

International Nuclear Information System (INIS)

Bernard, J.P.; Desert, X.

1990-01-01

Infrared Astronomy Satellite (IRAS) observations of the whole galaxy has shown that long wavelength emission (100 and 60 micron bands) can be explained by thermal emission from big grains (approx 0.1 micron) radiating at their equilibrium temperature when heated by the InterStellar Radiation Field (ISRF). This conclusion has been confirmed by continuum sub-millimeter observations of the galactic plane made by the EMILIE experiment at 870 microns (Pajot et al. 1986). Nevertheless, shorter wavelength observations like 12 and 25 micron IRAS bands, show an emission from the galactic plane in excess with the long wavelength measurements which can only be explained by a much hotter particles population. Because dust at equilibrium cannot easily reach high temperatures required to explain this excess, this component is thought to be composed of very small dust grains or big molecules encompassing thermal fluctuations. Researchers present here a numerical model that computes emission, from Near Infrared Radiation (NIR) to Sub-mm wavelengths, from a non-homogeneous spherical cloud heated by the ISRF. This model fully takes into account the heating of dust by multi-photon processes and back-heating of dust in the Visual/Infrared Radiation (VIS-IR) so that it is likely to describe correctly emission from molecular clouds up to large A sub v and emission from dust experiencing temperature fluctuations. The dust is a three component mixture of polycyclic aromatic hydrocarbons, very small grains, and classical big grains with independent size distributions (cut-off and power law index) and abundances

Multiplicity of pre-scission charged particle emission by a statistical model

International Nuclear Information System (INIS)

Matsuse, Takehiro

1996-01-01

With introducing the limitation (E cut-off ) not to excite all statistically permitted scission parts in the phase integral at the scission point, we try to reproduce the multiplicity of pre-scission charged particle emission of 86 Kr (E lab =890 MeV)+ 27 Al by the cascade calculation of the extended Hauser-Feshbach method (EHM). The physical image is explained from a point of view of the life time for the statistical model of the compound nuclei. When E cut-off parameter is bout 80 MeV, the cross section of scission and the loss of pre-scission charged particle seemed to be reproduced. The average pre-scission time is about 1.7 x 10 -20 sec. The essential problem of the life time of compound nuclei is explained. (S.Y.)

The resonance Bremsstrahlung of a fast charged particle in a medium

International Nuclear Information System (INIS)

Beshtoev, Kh.M.

1998-01-01

The Bremsstrahlung of the fast charged particle in the medium with dielectric permittivity ε at velocities υ ≥ c/n (n 2 =Reε) is considered. The Bremsstrahlung has singularity at β = 1/ncosθ (β = υ/c, θ is an angle of the Bremsstrahlung). This Bremsstrahlung is interpreted as resonance Bremsstrahlung with the width characterized by Imε=ε 2 , and the less ε 2 is, the higher the peak of this resonance rises. The angular distribution of the Bremsstrahlung is determined by cos θ=1/nβ and this angle coincides with the angle of the Cherenkov radiation. At β=1/n this resonance Bremsstrahlung goes in the forward direction and depends on frequency ω (ε=ε (ω))

Dynamical decay of nuclei at high temperature: competition between particle emission and fission decay

International Nuclear Information System (INIS)

Delagrange, H.; Gregoire, C.; Scheuter, F.; Abe, Y.

1985-06-01

A generalized diffusion equation is propounded to follow the time evolution of an excited nucleus towards fission including along the particle decay. This theoretical model is built in order to try to analyse the anomalous behaviour of particle emission observed in many experimental data for heavy-ion induced reactions. Some calculations for the systems 194 Hg, 170 Yb and 248 Cf are presented. A possible extension of this generalized formalism is suggested to deal more consistently with the experimental data. 52 refs. 10 figs.

Particle emissions from ventilation equipment: health hazards, measurement and product development; Ilmanvaihtolaitteiden hiukkaspaeaestoet: terveyshaitat, mittaaminen ja tuotekehitys

Energy Technology Data Exchange (ETDEWEB)

Tossavainen, A.; Tuovila, H.; Riala, R.; Harju, R.; Tuomi, T.; Voutilainen, R. [Tyoeterv.l, Helsinki (Finland); Laamanen, J.; Ismo Heimonen, I.; Kovanen, K. [VTT, Espoo (Finland)

2006-10-15

The project aimed to develop the design, structure and materials of ventilation equipment for the improvement of indoor air quality in office- type buildings. Particle emissions from commercial sound silencers were measured by laboratory tests. In ten buildings, the dust and fibre levels were surveyed in relation to the product design and operation. Direct-reading particle counters and filter sampling methods combined with optical and electron microscopy analyses were the main methods in these surveys. Nasal lavage was used for the estimation of inhalation exposure to coarse man-made mineral fibres. Technical criteria were drafted for the design and testing of fibre emissions from various ventilation equipment. (orig.)

Comprehensive Characterization Of Ultrafine Particulate Emission From 2007 Diesel Engines: PM Size Distribution, Loading And Indidividual Particle Size And Composition.

Science.gov (United States)

Zelenyuk, A.; Cuadra-Rodriguez, L. A.; Imre, D.; Shimpi, S.; Warey, A.

2006-12-01

The strong absorption of solar radiation by black carbon (BC) impacts the atmospheric radiative balance in a complex and significant manner. One of the most important sources of BC is vehicular emissions, of which diesel represents a significant fraction. To address this issue the EPA has issues new stringent regulations that will be in effect in 2007, limiting the amount of particulate mass that can be emitted by diesel engines. The new engines are equipped with aftertreatments that reduce PM emissions to the point, where filter measurements are subject to significant artifacts and characterization by other techniques presents new challenges. We will present the results of the multidisciplinary study conducted at the Cummins Technical Center in which a suite of instruments was deployed to yield comprehensive, temporally resolved information on the diesel exhaust particle loadings and properties in real-time: Particle size distributions were measured by Engine Exhaust Particle Sizer (EEPS) and Scanning Mobility Particle Sizer (SMPS). Total particle diameter concentration was obtained using Electrical Aerosol Detector (EAD). Laser Induced Incandescence and photoacoustic techniques were used to monitor the PM soot content. Single Particle Laser Ablation Time-of- flight Mass Spectrometer (SPLAT) provided the aerodynamic diameter and chemical composition of individual diesel exhaust particles. Measurements were conducted on a number of heavy duty diesel engines operated under variety of operating conditions, including FTP transient cycles, ramped-modal cycles and steady states runs. We have also characterized PM emissions during diesel particulate filter regeneration cycles. We will present a comparison of PM characteristics observed during identical cycles, but with and without the use of aftertreatment. A total of approximately 100,000 individual particles were sized and their composition characterized by SPLAT. The aerodynamic size distributions of the characterized

Modeling particle emission and power flow in pulsed-power driven, nonuniform transmission lines

Directory of Open Access Journals (Sweden)

Nichelle Bruner

2008-04-01

Full Text Available Pulsed-power driven x-ray radiographic systems are being developed to operate at higher power in an effort to increase source brightness and penetration power. Essential to the design of these systems is a thorough understanding of electron power flow in the transmission line that couples the pulsed-power driver to the load. In this paper, analytic theory and fully relativistic particle-in-cell simulations are used to model power flow in several experimental transmission-line geometries fielded on Sandia National Laboratories’ upgraded Radiographic Integrated Test Stand [IEEE Trans. Plasma Sci. 28, 1653 (2000ITPSBD0093-381310.1109/27.901250]. Good agreement with measured electrical currents is demonstrated on a shot-by-shot basis for simulations which include detailed models accounting for space-charge-limited electron emission, surface heating, and stimulated particle emission. Resonant cavity modes related to the transmission-line impedance transitions are also shown to be excited by electron power flow. These modes can drive oscillations in the output power of the system, degrading radiographic resolution.

How fast are the ultra-fast nano-scale solid-liquid phase transitions induced by energetic particles in solids?

International Nuclear Information System (INIS)

Lopasso, E.M.; Caro, A.; Caro, M.

2003-01-01

We study the thermodynamic forces acting on the evolution of the nanoscale regions excited by collisions of energetic particles into solid targets. We analyze the role of diffusion, thermo-migration, and the liquidus-solidus two-phase field crossing, as the system cools down from the collision-induced melt under different conditions of energy deposition. To determine the relevance of these thermodynamic forces, solute redistribution is evaluated using molecular dynamics simulations of equilibrium Au-Ni solid solutions. At low collision energies, our results show that the quenching of spherical cascades is too fast to allow for solute redistribution according to equilibrium solidification as determined from the equilibrium phase diagram (zone refining effect), and only thermo-migration is observed. At higher energies instead, in the cylindrical symmetry of ion tracks, quenching rate is in a range that shows the combined effects of thermo-migration and solute redistribution that, depending on the material, can reinforce or cancel each other. These results are relevant for the interpretation of the early stage of radiation damage in alloys, and show that the combination of ultra-fast but nano-scale characteristics of these processes can still be described in terms of linear response of the perturbed system

Development of solar flares and features of the fine structure of solar radio emission

Science.gov (United States)

Chernov, G. P.; Fomichev, V. V.; Yan, Y.; Tan, B.; Tan, Ch.; Fu, Q.

2017-11-01

The reason for the occurrence of different elements of the fine structure of solar radio bursts in the decimeter and centimeter wavelength ranges has been determined based on all available data from terrestrial and satellite observations. In some phenomena, fast pulsations, a zebra structre, fiber bursts, and spikes have been observed almost simultaneously. Two phenomena have been selected to show that the pulsations of radio emission are caused by particles accelerated in the magnetic reconnection region and that the zebra structure is excited in a source, such as a magnetic trap for fast particles. The complex combination of unusual fiber bursts, zebra structure, and spikes in the phenomenon on December 1, 2004, is associated with a single source, a magnetic island formed after a coronal mass ejection.

Investigating the Origins of Two Extreme Solar Particle Events: Proton Source Profile and Associated Electromagnetic Emissions

Energy Technology Data Exchange (ETDEWEB)

Kocharov, Leon; Usoskin, Ilya [Sodankylä Geophysical Observatory/Oulu Unit, University of Oulu, P.O.B. 3000, Oulu FI-90014 (Finland); Pohjolainen, Silja [Tuorla Observatory, University of Turku, Piikkiö FI-21500 (Finland); Mishev, Alexander [Space Climate Research Unit, University of Oulu, Oulu FI-90014 (Finland); Reiner, Mike J. [The Catholic University of America, Washington, DC, and NASA/Goddard Space Flight Center, Greenbelt, MD (United States); Lee, Jeongwoo [Department of Physics and Astronomy, Seoul National University, Seoul 151-747 (Korea, Republic of); Laitinen, Timo [Jeremiah Horrocks Institute, University of Central Lancashire, Preston PR1 2HE (United Kingdom); Didkovsky, Leonid V. [University of Southern California Space Sciences Center, 835 Bloom Walk, Los Angeles CA 90089 (United States); Pizzo, Victor J. [NOAA Space Weather Prediction Center, Boulder, CO 80305 (United States); Kim, Roksoon; Cho, Kyung-Suk [Korea Astronomy and Space Science Institute, Daejeon 305-348 (Korea, Republic of); Klassen, Andreas [Institut für Experimentelle und Angewandte Physik, Christian-Albrechts-Universität, Kiel D-24118 (Germany); Karlicky, Marian [Astronomical Institute of the Czech Academy of Sciences, Fričova 258, Ondřejov 251 65 (Czech Republic); Gary, Dale E. [Center for Solar-Terrestrial Research, New Jersey Institute of Technology, Newark NJ 07102-1982 (United States); Valtonen, Eino; Vainio, Rami [Space Research Laboratory, University of Turku, Turku FI-20014 (Finland)

2017-04-20

We analyze the high-energy particle emission from the Sun in two extreme solar particle events in which protons are accelerated to relativistic energies and can cause a significant signal even in the ground-based particle detectors. Analysis of a relativistic proton event is based on modeling of the particle transport and interaction, from a near-Sun source through the solar wind and the Earth’s magnetosphere and atmosphere to a detector on the ground. This allows us to deduce the time profile of the proton source at the Sun and compare it with observed electromagnetic emissions. The 1998 May 2 event is associated with a flare and a coronal mass ejection (CME), which were well observed by the Nançay Radioheliograph, thus the images of the radio sources are available. For the 2003 November 2 event, the low corona images of the CME liftoff obtained at the Mauna Loa Solar Observatory are available. Those complementary data sets are analyzed jointly with the broadband dynamic radio spectra, EUV images, and other data available for both events. We find a common scenario for both eruptions, including the flare’s dual impulsive phase, the CME-launch-associated decimetric-continuum burst, and the late, low-frequency type III radio bursts at the time of the relativistic proton injection into the interplanetary medium. The analysis supports the idea that the two considered events start with emission of relativistic protons previously accelerated during the flare and CME launch, then trapped in large-scale magnetic loops and later released by the expanding CME.

Ab-initio Pulsar Magnetosphere: Particle Acceleration in Oblique Rotators and High-energy Emission Modeling

Science.gov (United States)

Philippov, Alexander A.; Spitkovsky, Anatoly

2018-03-01

We perform global particle-in-cell simulations of pulsar magnetospheres, including pair production, ion extraction from the surface, frame-dragging corrections, and high-energy photon emission and propagation. In the case of oblique rotators, the effects of general relativity increase the fraction of the open field lines that support active pair discharge. We find that the plasma density and particle energy flux in the pulsar wind are highly non-uniform with latitude. A significant fraction of the outgoing particle energy flux is carried by energetic ions, which are extracted from the stellar surface. Their energies may extend up to a large fraction of the open field line voltage, making them interesting candidates for ultra-high-energy cosmic rays. We show that pulsar gamma-ray radiation is dominated by synchrotron emission, produced by particles that are energized by relativistic magnetic reconnection close to the Y-point and in the equatorial current sheet. In most cases, the calculated light curves contain two strong peaks, which is in general agreement with Fermi observations. The radiative efficiency decreases with increasing pulsar inclination and increasing efficiency of pair production in the current sheet, which explains the observed scatter in L γ versus \\dot{E}. We find that the high-frequency cutoff in the spectra is regulated by the pair-loading of the current sheet. Our findings lay the foundation for quantitative interpretation of Fermi observations of gamma-ray pulsars.

Self-consistent Study of Fast Particle Redistribution by Alfven Eigenmodes During Ion Cyclotron Resonance Heating

International Nuclear Information System (INIS)

Bergkvist, T.; Hellsten, T.; Johnson, T.

2006-01-01

Alfven eigenmodes (AEs) excited by fusion born α particles can degrade the heating efficiency of a burning plasma and throw out αs. To experimentally study the effects of excitation of AEs and the redistribution of the fast ions, ion cyclotron resonance heating (ICRH) is often used. The distribution function of thermonuclear αs in a reactor is expected to be isotropic and constantly renewed through DT reactions. The distribution function of cyclotron heated ions is strongly anisotropic, and the ICRH do not only renew the distribution function but also provide a strong decorrelation mechanism between the fast ions and the AE. Because of the sensitivity of the AE dynamics on the details of the distribution function, the location of the resonance surfaces in phase space and the extent of the overlapping resonant regions for different AEs, a self-consistent treatment of the AE excitation and the ICRH is necessary. Interactions of fast ions with AEs during ICRH has been implemented in the SELFO code. Simulations are in good agreement with the experimentally observer pitch-fork splitting and rapid damping of the AE as ICRH is turned off. The redistribution of fast ions have been studied in the presence of several driven AEs. (author)

Temperature and burning history affect emissions of greenhouse gases and aerosol particles from tropical peatland fire

Science.gov (United States)

Kuwata, Mikinori; Kai, Fuu Ming; Yang, Liudongqing; Itoh, Masayuki; Gunawan, Haris; Harvey, Charles F.

2017-01-01

Tropical peatland burning in Asia has been intensifying over the last decades, emitting huge amounts of gas species and aerosol particles. Both laboratory and field studies have been conducted to investigate emission from peat burning, yet a significant variability in data still exists. We conducted a series of experiments to characterize the gas and particulate matter emitted during burning of a peat sample from Sumatra in Indonesia. Heating temperature of peat was found to regulate the ratio of CH4 to CO2 in emissions (ΔCH4/ΔCO2) as well as the chemical composition of particulate matter. The ΔCH4/ΔCO2 ratio was larger for higher temperatures, meaning that CH4 emission is more pronounced at these conditions. Mass spectrometric analysis of organic components indicated that aerosol particles emitted at higher temperatures had more unsaturated bonds and ring structures than that emitted from cooler fires. The result was consistently confirmed by nuclear magnetic resonance analysis. In addition, CH4 emitted by burning charcoal, which is derived from previously burned peat, was lower by at least an order of magnitude than that from fresh peat. These results highlight the importance of both fire history and heating temperature for the composition of tropical peat-fire emissions. They suggest that remote sensing technologies that map fire histories and temperatures could provide improved estimates of emissions.

PIXE in 1980: Summary of the second international conference on particle induced x-ray emission and its analytical applications

International Nuclear Information System (INIS)

Akselsson, K.R.

1981-01-01

The Second International Conference on Particle Induced X-ray Emission (PIXE) and its analytical applications was held in Lund, Sweden, June 9-12, 1980. About a hundred papers were presented, including seven invited talks (PIXE and particle scattering, microbeam analysis, applications to aerosols and biological samples). The main impression left by the conference was that both the PIXE method and its applications are in a phase of fast development. Considerable effort has successfully been devoted to optimizing the basic PIXE technique. Also the great advantage of simultaneously getting information about lighter elements and sample mass was reported to have been successfully employed in routine analyses. PIXE, which was initially considered to be a method mainly for thin samples, has also been shown to be competitive for a variety of thick samples. Data from aerosol studies was presented. With the PIXE-method, it is feasible to perform series of measurements over a long period of time, many samples in parallel and/or samples from sites of poor accessibility. However, the advantages of PIXE may be further exploited in aerosol investigations and some promising lines of sampler development were reported. Sample preparation techniques are crucial for applications to biological samples and several laboratories are engaged in such developmental work. However, it was also evident that PIXE is already giving significant contributions to research in biology and medicine

Ultrafine particle emission characteristics of diesel engine by on-board and test bench measurement.

Science.gov (United States)

Huang, Cheng; Lou, Diming; Hu, Zhiyuan; Tan, Piqiang; Yao, Di; Hu, Wei; Li, Peng; Ren, Jin; Chen, Changhong

2012-01-01

This study investigated the emission characteristics of ultrafine particles based on test bench and on-board measurements. The bench test results showed the ultrafine particle number concentration of the diesel engine to be in the range of (0.56-8.35) x 10(8) cm(-3). The on-board measurement results illustrated that the ultrafine particles were strongly correlated with changes in real-world driving cycles. The particle number concentration was down to 2.0 x 10(6) cm(-3) and 2.7 x 10(7) cm(-3) under decelerating and idling operations and as high as 5.0 x 10(8) cm(-3) under accelerating operation. It was also indicated that the particle number measured by the two methods increased with the growth of engine load at each engine speed in both cases. The particle number presented a "U" shaped distribution with changing speed at high engine load conditions, which implies that the particle number will reach its lowest level at medium engine speeds. The particle sizes of both measurements showed single mode distributions. The peak of particle size was located at about 50-80 nm in the accumulation mode particle range. Nucleation mode particles will significantly increase at low engine load operations like idling and decelerating caused by the high concentration of unburned organic compounds.

Measurement of double differential cross sections of charged particle emission reactions by incident DT neutrons. Correction for energy loss of charged particle in sample materials

International Nuclear Information System (INIS)

Takagi, Hiroyuki; Terada, Yasuaki; Murata, Isao; Takahashi, Akito

2000-01-01

In the measurement of charged particle emission spectrum induced by neutrons, correcting the energy loss of charged particle in sample materials becomes a very important inverse problem. To deal with this inverse problem, we have applied the Bayesian unfolding method to correct the energy loss, and tested the performance of the method. Although this method is very simple, it was confirmed from the test that the performance was not inferior to other methods at all, and therefore the method could be a powerful tool for charged particle spectrum measurement. (author)

Fast inertial particle manipulation in oscillating flows

Science.gov (United States)

Thameem, Raqeeb; Rallabandi, Bhargav; Hilgenfeldt, Sascha

2017-05-01

It is demonstrated that micron-sized particles suspended in fluid near oscillating interfaces experience strong inertial displacements above and beyond the fluid streaming. Experiments with oscillating bubbles show rectified particle lift over extraordinarily short (millisecond) times. A quantitative model on both the oscillatory and the steady time scales describes the particle displacement relative to the fluid motion. The formalism yields analytical predictions confirming the observed scaling behavior with particle size and experimental control parameters. It applies to a large class of oscillatory flows with applications from particle trapping to size sorting.

Fast-ion stabilization of tokamak plasma turbulence

Science.gov (United States)

Di Siena, A.; Görler, T.; Doerk, H.; Poli, E.; Bilato, R.

2018-05-01

A significant reduction of the turbulence-induced anomalous heat transport has been observed in recent studies of magnetically confined plasmas in the presence of a significant fast-ion fractions. Therefore, the control of fast-ion populations with external heating might open the way to more optimistic scenarios for future fusion devices. However, little is known about the parameter range of relevance of these fast-ion effects which are often only highlighted in correlation with substantial electromagnetic fluctuations. Here, a significant fast ion induced stabilization is also found in both linear and nonlinear electrostatic gyrokinetic simulations which cannot be explained with the conventional assumptions based on pressure profile and dilution effects. Strong wave-fast particle resonant interactions are observed for realistic parameters where the fast particle trace approximation clearly failed and explained with the help of a reduced Vlasov model. In contrast to previous interpretations, fast particles can actively modify the Poisson field equation—even at low fast particle densities where dilution tends to be negligible and at relatively high temperatures, i.e. T  <  30T e . Further key parameters controlling the role of the fast ions are identified in the following and various ways of further optimizing their beneficial impact are explored. Finally, possible extensions into the electromagnetic regime are briefly discussed and the relevance of these findings for ITER standard scenarios is highlighted.

A fast and reliable method for computing free-bound emission coefficients for hydrogenic ions

International Nuclear Information System (INIS)

Sarmiento, A.; Canto, J.

1985-01-01

An approximate formula for the computation of the free-bound emission coefficient for hydrogenic ions is presented. The approximation is obtained through a manipulation of the (free-bound) Gaunt factor which intentionally distinguish the dependence on frequency from the dependence on temperature and ionic composition. Numerical tests indicate that the derived formula is very precise, fast and easy to use, making the calculation of the free-bound contribution from an ionized region of varying temperature and ionic composition a very simple and time-saving task. (author)

α particle induced scintillation in dense gaseous argon: emission spectra and temporal behavior of its ionic component

International Nuclear Information System (INIS)

Carvalho, M.J.; Klein, G.

1980-01-01

The scintillation induced by α particles in dense gaseous argon (above 1 atm) has been studied. The electric field dependence of the scintillation, shows that the second continuum (centred around 1270A) stems from the neutral as well as from the ionic species, initially created by the impinging particle. Intensity decay curves and emission spectra of these neutral excitation and ionic components were determined. Time constants suggest that the recombination mechanism is responsible for a delayed formation of the second continuum states, 1 Σ + sub(u) and 3 Σ + sub(u). The third continuum of the emission spectra, which spreads at longer wavelengths, from 1600A to 2800A, is field independent

Fast infrared detectors for beam diagnostics with synchrotron radiation

International Nuclear Information System (INIS)

Bocci, A.; Marcelli, A.; Pace, E.; Drago, A.; Piccinini, M.; Cestelli Guidi, M.; De Sio, A.; Sali, D.; Morini, P.; Piotrowski, J.

2007-01-01

Beam diagnostic is a fundamental constituent of any particle accelerators either dedicated to high-energy physics or to synchrotron radiation experiments. All storage rings emit radiations. Actually they are high brilliant sources of radiation: the synchrotron radiation emission covers from the infrared range to the X-ray domain with a pulsed structure depending on the temporal characteristics of the stored beam. The time structure of the emitted radiation is extremely useful as a tool to perform time-resolved experiments. However, this radiation can be also used for beam diagnostic to determine the beam stability and to measure the dimensions of the e - or e + beam. Because of the temporal structure of the synchrotron radiation to perform diagnostic, we need very fast detectors. Indeed, the detectors required for the diagnostics of the stored particle bunches at third generation synchrotron radiation sources and FEL need response times in the sub-ns and even ps range. To resolve the bunch length and detect bunch instabilities, X-ray and visible photon detectors may be used achieving response times of a few picoseconds. Recently, photon uncooled infrared devices optimized for the mid-IR range realized with HgCdTe semiconductors allowed to obtain sub-nanosecond response times. These devices can be used for fast detection of intense IRSR sources and for beam diagnostic. We present here preliminary experimental data of the pulsed synchrotron radiation emission of DAΦNE, the electron positron collider of the LNF laboratory of the INFN, performed with new uncooled IR detectors with a time resolution of a few hundreds of picoseconds

Delayed Proton Emission in the A=70 Region, a Strobe for Level Density and Particle Width

CERN Multimedia

2002-01-01

The delayed particle emission, which is a characteristic signature of the most exotic nuclei decay, provides a wide variety of spectroscopic information among which level density, and gives in some cases access to selected microscopic structures. In regard to these two aspects the $\\beta^+$-EC delayed proton emission in the A=70 neutron deficient mass region is of special interest to be investigated. Indeed, in this area located close to the proton drip line and along the N=Z line, the delayed proton emission constitutes an access to level density in the Q$_{EC}$-S$_p$ window of the emitting nucleus. Moreover, the unbound states populated by the EC process are expected to exhibit lifetimes in the vicinity of the K electronic shell filling time ($\\tau\\!\\sim\\!2\\times10^{-16}$s) and so the particle widths can be reached via proton X-ray coincidence measurements (PXCT). From theoretical approaches strongly deformed low-spin proton unbound levels which may be populated in the T$_Z$ = 1/2 precursors decay are predi...

Films with discrete nano-DLC-particles as the field emission cascade

International Nuclear Information System (INIS)

Song Fengqi; Bu Haijun; Wan Jianguo; Wang Guanghou; Zhou Feng; He Longbing; Han Min; Zhou Jianfeng; Wang Xiaoshu

2008-01-01

Films with discrete diamond-like-carbon (DLC) nanoparticles were prepared by the deposition of the carbon nanoparticle beam. Their morphologies were imaged by scanning electron microscopy and atomic force microscopy (AFM). The nanoparticles were found to be distributed on the silicon (1 0 0) substrate discretely. Hemispherical shapes of the nanoparticles were demonstrated by the AFM line profile. Electron energy loss spectra were measured and an sp 3 ratio as high as 86% was found. Field-induced electron emission of the as-prepared cascade (nanoDLC/ Si) was tested and a current density of 1 mA cm -2 was achieved at 10.2 V μm -1 . (fast track communication)

Proceedings of International Symposium TEPA 2015: Thunderstorms and Elementary Particle Acceleration

International Nuclear Information System (INIS)

Chilingarian, A.

2016-03-01

The problem of how lightning is initiated inside thunderclouds is probably one of the biggest mysteries in the atmospheric sciences. Recently established high energy processes in the atmosphere, i.e. Terrestrial Gamma Flashes (TGF) – brief bursts of gamma rays observed by orbiting gamma ray observatories and Thunderstorm Ground Enhancements (TGEs) – sizable long-lasting fluxes of electrons, gamma rays and neutrons detected on Earth’s surface are correlated with thunderstorms. However, the relationship among thundercloud electrification, lightning activity, and wideband radio emission and enhanced particle fluxes have not been yet unambiguously established. One of the most intriguing opportunities opened by the observation of the high-energy processes in the atmosphere is their relation to lightning initiation and propagation. Lightning discharges and TGEs are alternative mechanisms for the discharging of the atmospheric “electric engine” and synchronized observations of both phenomena help to understand them better. With the objective to discuss these high-energy phenomena, the conference on Thunderstorms and Elementary Particle Acceleration was held at the Nor Amberd International Conference Center of the Yerevan Physics Institute (YerPhI) in Armenia. The Cosmic Ray Division of the YerPhI and Skobeltsyn Institute of Nuclear Physics of Moscow State University organized the workshop; YerPhI and the Armenian State Committee of Science sponsored it. Thirty scientists and students from the United States, Japan, France, Germany, Israel, Russia, and Armenia attended. Presentations focused on observations and models of high-energy emissions in thunderclouds; on the termination of particle fluxes by lightning; multivariate observations of thunderstorms from the Earth’s surface and from space; radio emissions produced by atmospheric discharges and particle fluxes; the influence of the Extensive Air Showers (EASes) on lightning initiation and others. Discussions

Time dependent emission line profiles in the radially streaming particle model of Seyfert galaxy nuclei and quasi-stellar objects

Science.gov (United States)

Hubbard, R.

1974-01-01

The radially-streaming particle model for broad quasar and Seyfert galaxy emission features is modified to include sources of time dependence. The results are suggestive of reported observations of multiple components, variability, and transient features in the wings of Seyfert and quasi-stellar emission lines.

α-cluster model for the multiple emission of particles in the reaction 90Zr (e, α)

International Nuclear Information System (INIS)

Guevara, Y.M.; Garcia, C.; Hoyos, O.E.R.; Rodriguez, T. E.; Arruda-Neto, J.D.T.

2011-01-01

We present a methodology based on the model of photoabsorption by a cluster N- α for a better understanding of the puzzling steady increase behavior of the 90 Zr (e, α) yield obtained experimentally in the energy range of the giant dipole resonance (RDG) and the quasi-deuteron (QD).The calculation takes into account the emission of protons, neutrons and alpha particles in the framework of the reaction (which was used for the Intranuclear Cascade model (MCMC)). The statistical decay of the compound nucleus is described by Monte Carlo techniques in terms of competition between evaporation of particles (p, n, d, α, 3 He t) and nuclear fission, but for our specific case (the reaction and + Zr 90 in an energy range between 20 and 140 MeV) the fission channel does not have a high probability of occurrence. The results reproduce quite successfully the experimental data, suggesting that pre-equilibrium emission of alpha particles are essential for the interpretation of this exotic increase of the cross sections. (Author)

Fast numerical method for solving the three-dimensional Stokes' equations in the presence of suspended particles

International Nuclear Information System (INIS)

Fogelson, A.L.; Peskin, C.S.

1988-01-01

A new fast numerical method for solving the three-dimensional Stokes' equations in the presence of suspended particles is presented. The fluid dynamics equations are solved on a lattice. A particle is represented by a set of points each of which moves at the local fluid velocity and is not constrained to lie on the lattice. These points are coupled by forces which resist deformation of the particle. These forces contribute to the force density in the Stokes' equations. As a result, a single set of fluid dynamics equations holds at all points of the domain and there are no internal boundaries. Particles size, shape, and deformability may be prescribed. Computational work increases only linearly with the number of particles, so large numbers (500--1000) of particles may be studied efficiently. The numerical method involves implicit calculation of the particle forces by minimizing an energy function and solution of a finite-difference approximation to the Stokes' equations using the Fourier--Toeplitz method. The numerical method has been implemented to run on all CRAY computers: the implementation exploits the CRAY's vectorized arithmetic, and on machines with insufficient central memory, it performs efficient disk I/O while storing most of the data on disk. Applications of the method to sedimentation of one-, two-, and many-particle systems are described. Trajectories and settling speeds for two-particle sedimentation, and settling speed for multiparticle sedimentation from initial distributions on a cubic lattice or at random give good quantitative agreement with existing theories. copyright 1988 Academic Press, Inc

Design of Slow and Fast Light Photonic Crystal Waveguides for Single-photon Emission Using a Bloch Mode Expansion Technique

DEFF Research Database (Denmark)

de Lasson, Jakob Rosenkrantz; Rigal, B.; Kapon, E.

We design slow and fast light photonic crystal waveguides for single-photon emission using a Bloch mode expansion and scattering matrix technique. We propose slow light designs that increase the group index-waveguide mode volume ratio for larger Purcell enhancement, and address efficient slow-to-...

Quantum 1/f noise in non-degerate semiconductors and emission statistics of alpha particles

International Nuclear Information System (INIS)

Kousik, G.S.

1985-01-01

Charged particle scattering is accompanied by the emission of soft photons. Handel's theory of 1/f noise, based on the infrared divergent coupling of the system to the electromagnetic field or other elementary excitations, states that the current associated with a beam of scattered particles will exhibit 1/f noise. The fraction of the particles scattered with an energy loss epsilon to soft photon emission is proportional to 1/epsilon and herein lies the origin of the quantum theory of 1/f noise. The 1/f noise caused by mobility fluctuations in semiconductors is related to the scattering cross section fluctuation given by Handel's theory, through the relaxation time. Chapters Two through Five of this dissertation presents the results of the detailed calculation of mobility fluctuation 1/f noise and Hooge parameter in nondegenerate semiconductors. Numerical results are given for silicon and gallium arsenide. Data obtained from extensive measurements on counting techniques for alpha-particles radioactive decay from a source containing 94 Pu 239 , 95 Am 241 and 96 Cm 244 are presented in Chapters Six and Seven of this dissertation. These data show that the statistics are non-Poissonian for large counting times (of the order of 1000 minutes) contrary to the popular belief that alpha-decay is an example of Poissonian statistics. Measurements of the Allan variance indicated the presence of a slow Lorentzian flicker noise and 1/f noise and the magnitude of the noise for large counting times is considerably larger than that predicted by Poissonian statistics

The effect of dynamic operating conditions on nano-particle emissions from a light-duty diesel engine applicable to prime and auxiliary machines on marine vessels

Directory of Open Access Journals (Sweden)

Hyungmin Lee

2012-12-01

Full Text Available This study presents the nano-sized particle emission characteristics from a small turbocharged common rail diesel engine applicable to prime and auxiliary machines on marine vessels. The experiments were conducted under dynamic engine operating conditions, such as steady-state, cold start, and transient conditions. The particle number and size distributions were analyzed with a high resolution PM analyzer. The diesel oxidation catalyst (DOC had an insignificant effect on the reduction in particle number, but particle number emissions were drastically reduced by 3 to 4 orders of magnitude downstream of the diesel particulate filter (DPF at various steady conditions. Under high speed and load conditions, the particle filtering efficiency was decreased by the partial combustion of trapped particles inside the DPF because of the high exhaust temperature caused by the increased particle number concentration. Retarded fuel injection timing and higher EGR rates led to increased particle number emissions. As the temperature inside the DPF increased from 25 °C to 300 °C, the peak particle number level was reduced by 70% compared to cold start conditions. High levels of nucleation mode particle generation were found in the deceleration phases during the transient tests.

ITER Plasma at Ion Cyclotron Frequency Domain: The Fusion Alpha Particles Diagnostics Based on the Stimulated Raman Scattering of Fast Magnetosonic Wave off High Harmonic Ion Bernstein Modes

Science.gov (United States)

Stefan, V. Alexander

2014-10-01

A novel method for alpha particle diagnostics is proposed. The theory of stimulated Raman scattering, SRS, of the fast wave and ion Bernstein mode, IBM, turbulence in multi-ion species plasmas, (Stefan University Press, La Jolla, CA, 2008). is utilized for the diagnostics of fast ions, (4)He (+2), in ITER plasmas. Nonlinear Landau damping of the IBM on fast ions near the plasma edge leads to the space-time changes in the turbulence level, (inverse alpha particle channeling). The space-time monitoring of the IBM turbulence via the SRS techniques may prove efficient for the real time study of the fast ion velocity distribution function, spatial distribution, and transport. Supported by Nikola Tesla Labs., La Jolla, CA 92037.

Particle emissions from ventilation equipment: health hazards, measurement and product development; Ilmanvaihtolaitteiden hiukkaspaeaestoet: terveyshaitat, mittaaminen ja tuotekehitys - ILMI

Energy Technology Data Exchange (ETDEWEB)

Tossavainen, A.; Paananen, H.; Riala, R.; Tuomi, T.; Voutilainen, R. [Finnish Institute of Occupational Health, Helsinki (Finland); Heimonen, I.; Kovanen, K. [VTT Building and Transport, Espoo (Finland)

2004-07-01

The project will develop the design, structure and materials of ventilation equipment for the improvement of indoor air quality in office-type buildings. Particle emissions from commercial products are measured by laboratory tests. In ten buildings, the dust and fibre levels will be surveyed in relation to the design and operation of the ventilation equipment. Direct-reading particle counters and filter sampling method combined with optical and electron microscopy analyses are the main methods in these surveys. Nasal lavage is used for the estimation of inhalation exposure to coarse man-made mineral fibres. Technical criteria will be drafted for the design and testing of fibre emissions from various ventilation equipment. (orig.)

Enhanced emission of non-compound light particles in the reaction plane

International Nuclear Information System (INIS)

Tsang, M.B.

1984-01-01

In an experiment performed at the K500 cyclotron at Michigan State University, light particles in coincidence with two fission fragments for 14 N induced reactions on 197 Au at 420 MeV incident energy have been measured. The fission fragments were detected with two large area position sensitive parallel plate avalanche detectors. Light particle telescopes consisting of silicon-ΔE and Nal-E detectors were placed both in and out of the plane defined by the centers of the two fission detectors and the beam axis. The momentum transferred to the composite system was determined by measuring the folding angle between the two outgoing fission fragments. Unlike observations with more fissile targets, however, transfer and inelastic reactions characterized by small linear momentum transfers contribute negligibly to the fission cross section for reactions on the 197 Au target. For events which lead to fission, the most probable linear momentum transfer corresponded to about 85% of the beam momentum. This is similar to the most probable momentum transfer observed for fusion-like reactions on 238 U at the same beam energy. Much of the missing momentum is carried away by non-equilibrium light particle emission

Neutral particle balance in GDT with fast titanium coating of the first wall

International Nuclear Information System (INIS)

Bagryansky, P.A.; Bender, E.D.; Ivanov, A.A.; Krahl, S.; Noack, K.; Karpushov, A.N.; Murakhtin, S.V.; Shikhovtsev, I.V.

1995-01-01

The GDT is an axisymmetric open trap with a high mirror ratio for confinement of a collisional plasma. The experimental program of the GDT was focused on the generation of plasma physics database necessary for a GDT-based neutron source. A distinct feature of both GDT and the GDT-based neutron source is that the Larmor radius of the fast sloshing ions is comparable to plasma radius. In this case, the sloshing ions can not be well shielded by the plasma halo from penetration of the neutral gas from periphery that results in high charge exchange losses. The plasma parameters are then very sensitive to gas pressure near the plasma boundary. To reduce the gas pressure to desured value during the beam heating, the authors have used arc-type evaporators developed at the Budker INP for fast titanium coating of the GDT first wall. If needed, the coating can be done a few seconds before each shot. They investigated the neutral particle balance in presence of NB-heating. The inverted magnetron gauges were used to study the temporal dependence of gas pressure inside the central cell. Pyroelectric bolometers were employed to measure the flux of charge exchange neutrals. Neutral particle balance has also been studied numerically by using a gas-transport code. The results of the investigations are the following: (1) sloshing ion lifetime was increased about 10 times compared to that without the coating of the first wall; and (2) wall recycling coefficient of the Ti-coated wall does not exceed 1 for 8 keV mean energy of the neutral hydrogen atoms striking the wall

Compaction of a Bed of Fragmentable Particles and Associated Acoustic Emission

International Nuclear Information System (INIS)

Hegron, L.; Sornay, P.; Favretto-Cristini, N.

2013-06-01

The nuclear fuel of light water power reactors are manufactured by powder metallurgy. This is also the method that is used for the production of fuels containing minor actinides that have high activity and long life. Given their radiotoxicity, it is necessary to simplify the manufacturing process to the maximum, limiting dissemination and retention of matter. In addition, the fuel must have a mostly open porosity. Implementation of particles of a few hundred micrometers and controlled cohesion could meet this dual objective. However, it should be ensured that the mechanical strength of compacts before sintering is sufficient without adding binder. The phenomena that occur during the manufacture of compact are thus analyzed and quantified. It is shown that only a portion of the particles breaks upon application of a stress up to 600 MPa and it is possible to detect this fragmentation by acoustic emission (AE). (authors)

4-Nitrophenol, 1-nitropyrene, and 9-nitroanthracene emissions in exhaust particles from diesel vehicles with different exhaust gas treatments

Science.gov (United States)

Inomata, Satoshi; Fushimi, Akihiro; Sato, Kei; Fujitani, Yuji; Yamada, Hiroyuki

2015-06-01

The dependence of nitro-organic compound emissions in automotive exhaust particles on the type of aftertreatment used was investigated. Three diesel vehicles with different aftertreatment systems (an oxidation catalyst, vehicle-DOC; a particulate matter and NOx reduction system, vehicle-DPNR; and a urea-based selective catalytic reduction system, vehicle-SCR) and a gasoline car with a three-way catalyst were tested. Nitro-polycyclic aromatic hydrocarbons (nitro-PAHs) and nitrophenols in the particles emitted were analyzed by thermal desorption gas chromatography/mass spectrometry and liquid chromatography/mass spectrometry. The secondary production of nitro-organic compounds on the filters used to collect particles and the adsorption of gaseous nitro-organic compounds by the filters were evaluated. Emissions of 1-nitropyrene, 9-nitroanthracene, and 4-nitrophenol in the diesel exhaust particles were then quantified. The NOx reduction process in vehicle-DPNR appeared to remove nitro-hydrocarbons efficiently but not to remove nitro-oxygenated hydrocarbons efficiently. The nitro-PAH emission factors were lower for vehicle-DOC when it was not fitted with a catalyst than when it was fitted with a catalyst. The 4-nitrophenol emission factors were also lower for vehicle-DOC with a catalyst than vehicle-DOC without a catalyst, suggesting that the oxidation catalyst was a source of both nitro-PAHs and 4-nitrophenol. The time-resolved aerosol mass spectrometry data suggested that nitro-organic compounds are mainly produced when an engine is working under load. The presence of 4-nitrophenol in the particles was not confirmed statistically because of interference from gaseous 4-nitrophenol. Systematic errors in the estimated amounts of gaseous 1-nitropyrene and 9-nitroanthracene adsorbed onto the filters and the estimated amounts of volatile nitro-organic compounds that evaporated during sampling and during post-sampling conditioning could not be excluded. An analytical method

Sub-millisecond electron density profile measurement at the JET tokamak with the fast lithium beam emission spectroscopy system

Science.gov (United States)

Réfy, D. I.; Brix, M.; Gomes, R.; Tál, B.; Zoletnik, S.; Dunai, D.; Kocsis, G.; Kálvin, S.; Szabolics, T.; JET Contributors

2018-04-01

Diagnostic alkali atom (e.g., lithium) beams are routinely used to diagnose magnetically confined plasmas, namely, to measure the plasma electron density profile in the edge and the scrape off layer region. A light splitting optics system was installed into the observation system of the lithium beam emission spectroscopy diagnostic at the Joint European Torus (JET) tokamak, which allows simultaneous measurement of the beam light emission with a spectrometer and a fast avalanche photodiode (APD) camera. The spectrometer measurement allows density profile reconstruction with ˜10 ms time resolution, absolute position calculation from the Doppler shift, spectral background subtraction as well as relative intensity calibration of the channels for each discharge. The APD system is capable of measuring light intensities on the microsecond time scale. However ˜100 μs integration is needed to have an acceptable signal to noise ratio due to moderate light levels. Fast modulation of the beam up to 30 kHz is implemented which allows background subtraction on the 100 μs time scale. The measurement covers the 0.9 background subtraction, the relative calibration, and the comprehensive error calculation, runs a Bayesian density reconstruction code, and loads results to the JET database. The paper demonstrates the capability of the APD system by analyzing fast phenomena like pellet injection and edge localized modes.

Fast rise time IR detectors for lepton colliders

International Nuclear Information System (INIS)

Drago, A.; Bini, S.; Guidi, M. Cestelli; Marcelli, A.; Pace, E.

2016-01-01

Diagnostics is a fundamental issue for accelerators whose demands are continuously increasing. In particular bunch-by-bunch diagnostics is a key challenge for the latest generation of lepton colliders and storage rings. The Frascati Φ-factory, DAΦNE, colliding at 1.02 GeV in the centre of mass, hosts in the main rings few synchrotron radiation beamlines and two of them collect the synchrotron radiation infrared emission: SINBAD from the electron ring and 3+L from the positron ring. At DAΦNE each bucket is 2.7 ns long and particles are gathered in bunches emitting pulsed IR radiation, whose intensity in the long wavelength regime is directly proportional to the accumulated particles. Compact uncooled photoconductive HgCdTe detectors have been tested in both beamlines using dedicated optical layouts. Actually, the fast rise time of HgCdTe semiconductors give us the chance to test bunch-by-bunch devices for both longitudinal and transverse diagnostics. For the longitudinal case, single pixel detectors have been used, while for the transverse diagnostics, multi-pixel array detectors, with special custom design, are under test. This contribution will briefly describe the status of the research on fast IR detectors at DAΦNE, the results obtained and possible foreseen developments.

Qualitative analysis of a powdered diamond sample by particle induced X-ray emission (PIXE)

International Nuclear Information System (INIS)

Mabida, C.; Annegarn, H.J.; Renan, M.J.; Sellschop, J.P.F.

The main purpose of this analysis was to determine whether nickel is present in diamond powder as a trace element. Particle induced X-ray emission (PIXE) showed unambiguously that nickel was present. Due to the convenience of PIXE in multielemental analysis, the investigations also include a number of other trace elements in the sample

Gamma-ray emission from internal shocks in novae

Science.gov (United States)

Martin, P.; Dubus, G.; Jean, P.; Tatischeff, V.; Dosne, C.

2018-04-01

Context. Gamma-ray emission at energies ≥100 MeV has been detected from nine novae using the Fermi Large Area Telescope (LAT), and can be explained by particle acceleration at shocks in these systems. Eight out of these nine objects are classical novae in which interaction of the ejecta with a tenuous circumbinary material is not expected to generate detectable gamma-ray emission. Aim. We examine whether particle acceleration at internal shocks can account for the gamma-ray emission from these novae. The shocks result from the interaction of a fast wind radiatively-driven by nuclear burning on the white dwarf with material ejected in the initial runaway stage of the nova outburst. Methods: We present a one-dimensional model for the dynamics of a forward and reverse shock system in a nova ejecta, and for the associated time-dependent particle acceleration and high-energy gamma-ray emission. Non-thermal proton and electron spectra are calculated by solving a time-dependent transport equation for particle injection, acceleration, losses, and escape from the shock region. The predicted emission is compared to LAT observations of V407 Cyg, V1324 Sco, V959 Mon, V339 Del, V1369 Cen, and V5668 Sgr. Results: The ≥100 MeV gamma-ray emission arises predominantly from particles accelerated up to 100 GeV at the reverse shock and undergoing hadronic interactions in the dense cooling layer downstream of the shock. The emission rises within days after the onset of the wind, quickly reaches a maximum, and its subsequent decrease reflects mostly the time evolution of the wind properties. Comparison to gamma-ray data points to a typical scenario where an ejecta of mass 10-5-10-4 M⊙ expands in a homologous way with a maximum velocity of 1000-2000 km s-1, followed within a day by a wind with a velocity values of which result in the majority of best-fit models having gamma-ray spectra with a high-energy turnover below 10 GeV. Our typical model is able to account for the main

A Cherenkov-emission Microwave Source*

Science.gov (United States)

Lai, C. H.; Yoshii, J.; Katsouleas, T.; Hairapetian1, G.; Joshi, C.; Mori, W.

1996-11-01

In an unmagnetized plasma, there is no Cherenkov emission because the phase velocity vf of light is greater than c. In a magnetized plasma, the situation is completely changed. There is a rich variety of plasma modes with phase velocities vf 2 c which can couple to a fast particle. In the magnetized plasma, a fast particle, a particle beam, or even a short laser pulse excites a Cherenkov wake that has both electrostatic and electromagnetic components. Preliminary simulations indicate that at the vacuum/plasma boundary, the wake couples to a vacuum microwave with an amplitude equal to the electromagnetic component in the plasma. For a weakly magnetized plasma, the amplitude of the out-coupled radiation is approximately wc/wp times the amplitude of the wake excited in the plasma by the beam, and the frequency is approximately wp. Since plasma wakes as high as a few GeV/m are produced in current experiments, the potential for a high-power (i.e., GWatt) coherent microwave to THz source exists. In this talk, a brief overview of the scaling laws will be presented, followed by 1-D and 2-D PIC simulations. Prospects for a tuneable microwave source experiment based on this mechanism at the UCLA plasma wakefield accelerator facility will be discussed. *Work supported by AFOSR Grant #F4 96200-95-0248 and DOE Grant # DE-FG03-92ER40745. 1Now at Hughes Research Laboratories, Malibu, CA 90265

Error estimation and parameter dependence of the calculation of the fast ion distribution function, temperature, and density using data from the KF1 high energy neutral particle analyzer on Joint European Torus

International Nuclear Information System (INIS)

Schlatter, Christian; Testa, Duccio; Cecconello, Marco; Murari, Andrea; Santala, Marko

2004-01-01

Joint European Torus high energy neutral particle analyzer measures the flux of fast neutrals originating from the plasma core. From this data, the fast ion distribution function f i fast , temperature T i,perpendicular fast , and density n i fast are derived using knowledge of various plasma parameters and of the cross section for the required atomic processes. In this article, a systematic sensitivity study of the effect of uncertainties in these quantities on the evaluation of the neutral particle analyzer f i fast , T i,perpendicular fast , and n i fast is reported. The dominant parameter affecting n i fast is the impurity confinement time and therefore a reasonable estimate of this quantity is necessary to reduce the uncertainties in n i fast below 50%. On the other hand, T i,perpendicular fast is much less sensitive and can certainly be provided with an accuracy of better than 10%

Aerosol particle mixing state, refractory particle number size distributions and emission factors in a polluted urban environment: Case study of Metro Manila, Philippines

Science.gov (United States)

Kecorius, Simonas; Madueño, Leizel; Vallar, Edgar; Alas, Honey; Betito, Grace; Birmili, Wolfram; Cambaliza, Maria Obiminda; Catipay, Grethyl; Gonzaga-Cayetano, Mylene; Galvez, Maria Cecilia; Lorenzo, Genie; Müller, Thomas; Simpas, James B.; Tamayo, Everlyn Gayle; Wiedensohler, Alfred

2017-12-01

Ultrafine soot particles (black carbon, BC) in urban environments are related to adverse respiratory and cardiovascular effects, increased cases of asthma and premature deaths. These problems are especially pronounced in developing megacities in South-East Asia, Latin America, and Africa, where unsustainable urbanization ant outdated environmental protection legislation resulted in severe degradation of urban air quality in terms of black carbon emission. Since ultrafine soot particles do often not lead to enhanced PM10 and PM2.5 mass concentration, the risks related to ultrafine particle pollution may therefore be significantly underestimated compared to the contribution of secondary aerosol constituents. To increase the awareness of the potential toxicological relevant problems of ultrafine black carbon particles, we conducted a case study in Metro Manila, the capital of the Philippines. Here, we present a part of the results from a detailed field campaign, called Manila Aerosol Characterization Experiment (MACE, 2015). Measurements took place from May to June 2015 with the focus on the state of mixing of aerosol particles. The results were alarming, showing the abundance of externally mixed refractory particles (soot proxy) at street site with a maximum daily number concentration of approximately 15000 #/cm3. That is up to 10 times higher than in cities of Western countries. We also found that the soot particle mass contributed from 55 to 75% of total street site PM2.5. The retrieved refractory particle number size distribution appeared to be a superposition of 2 ultrafine modes at 20 and 80 nm with a corresponding contribution to the total refractory particle number of 45 and 55%, respectively. The particles in the 20 nm mode were most likely ash from metallic additives in lubricating oil, tiny carbonaceous particles and/or nucleated and oxidized organic polymers, while bigger ones (80 nm) were soot agglomerates. To the best of the authors' knowledge, no other

Particle induced X-ray emission and complementary nuclear methods for trace element determination; Plenary lecture

Energy Technology Data Exchange (ETDEWEB)

Johansson, S A.E. [Lund Univ. (Sweden). Dept. of Nuclear Physics

1992-03-01

In this review the state-of-the-art of particle induced X-ray emission (PIXE) methods for the determination of trace elements is described. The developmental work has mostly been carried out in nuclear physics laboratories, where accelerators are available, but now the increased interest has led to the establishment of other dedicated PIXE facilities. The reason for this interest is the versatility, high sensitivity and multi-element capability of PIXE analysis. A further very important advantage is that PIXE can be combined with the microbeam technique, which makes elemental mapping with a spatial resolution of about 1 {mu}m possible. As a technique, PIXE can also be combined with other nuclear reactions such as elastic scattering and particle-induced gamma emission, so that light elements can be determined. The usefulness of PIXE is illustrated by a number of typical applications in biology, medicine, geology, air pollution research, archaeology and the arts. (author).

Light charged particle production induced by fast neutrons (En=25-65 MeV) on 209Bi

International Nuclear Information System (INIS)

Raeymackers, Erwin; Slypen, Isabelle; Benck, Sylvie; Meulders, Jean-Pierre; Nica, Ninel; Corcalciuc, Valentin

2002-01-01

This paper presents the experimental set-up and data reduction procedures regarding the measurement of double-differential cross sections for light charged particle production in fast neutron induced reactions (n, px), (n, dx), (n, tx) and (n, αx) on bismuth in the incident neutron energy range 25-65 MeV and at laboratory angles from 20deg to 160deg. preliminary double-differential and energy-differential cross sections for hydrogen isotopes are presented. (author)

Particle filtering based structural assessment with acoustic emission sensing

Science.gov (United States)

Yan, Wuzhao; Abdelrahman, Marwa; Zhang, Bin; Ziehl, Paul

2017-02-01

Nuclear structures are designed to withstand severe loading events under various stresses. Over time, aging of structural systems constructed with concrete and steel will occur. This deterioration may reduce service life of nuclear facilities and/or lead to unnecessary or untimely repairs. Therefore, online monitoring of structures in nuclear power plants and waste storage has drawn significant attention in recent years. Of many existing non-destructive evaluation and structural monitoring approaches, acoustic emission is promising for assessment of structural damage because it is non-intrusive and is sensitive to corrosion and crack growth in reinforced concrete elements. To provide a rapid, actionable, and graphical means for interpretation Intensity Analysis plots have been developed. This approach provides a means for classification of damage. Since the acoustic emission measurement is only an indirect indicator of structural damage, potentially corrupted by non-genuine data, it is more suitable to estimate the states of corrosion and cracking in a Bayesian estimation framework. In this paper, we will utilize the accelerated corrosion data from a specimen at the University of South Carolina to develop a particle filtering-based diagnosis and prognosis algorithm. Promising features of the proposed algorithm are described in terms of corrosion state estimation and prediction of degradation over time to a predefined threshold.

First- and second-chance proton emission in the interactions of fast neutrons with 92Mo

International Nuclear Information System (INIS)

Qaim, S.M.; Wolfle, R.; Strohmaier, B.

1989-01-01

Cross sections were measured radiochemically for the 92 Mo(n,p) 92 Nb m and 92 Mo(n,n'p +pn+d) 91 Nb m reactions over the neutron energy range of 9.0--10.6 MeV, and for the latter reaction also between 12.6 and 14.4 MeV. Use was made of high-resolution γ-ray and x-ray spectroscopy. Statistical-model calculations taking into account precompound effects were performed for fast neutron induced reactions on 92 Mo. The calculational results agree well with the experimental data on emitted proton spectra as well as on the excitation functions of various reaction channels. The second-chance proton emission is significant for incident neutron energies above 11 MeV; between 13 and 14 MeV it is comparable to the first-chance proton emission

Effects of Particle Filters and Selective Catalytic Reduction on In-Use Heavy-Duty Diesel Truck Emissions

Science.gov (United States)

Preble, C.; Cados, T.; Harley, R.; Kirchstetter, T.

2016-12-01

Heavy-duty diesel trucks (HDDT) are a major source of nitrogen oxides (NOx) and black carbon (BC) in urban environments, contributing to persistent ozone and particulate matter air quality problems. Diesel particle filters (DPFs) and selective catalytic reduction (SCR) systems that target PM and NOx emissions, respectively, have recently become standard equipment on new HDDT. DPFs can also be installed on older engines as a retrofit device. Previous work has shown that DPF and SCR systems can reduce NOx and BC emissions by up to 70% and 90%, respectively, compared to modern trucks without these after-treatment controls (Preble et al., ES&T 2015). DPFs can have the undesirable side-effect of increasing ultrafine particle (UFP) and nitrogen dioxide (NO2) emissions. While SCR systems can partially mitigate DPF-related NO2 increases, these systems can emit nitrous oxide (N2O), a potent greenhouse gas. We report new results from a study of HDDT emissions conducted in fall 2015 at the Port of Oakland and Caldecott Tunnel in California's San Francisco Bay Area. We report pollutant emission factors (g kg-1) for emitted NOx, NO2, BC, PM2.5, UFP, and N2O on a truck-by-truck basis. Using a roadside license plate recognition system, we categorize each truck by its engine model year and installed after-treatment controls. From this, we develop emissions profiles for trucks with and without DPF and SCR. We evaluate the effectiveness of these devices as a function of their age to determine whether degradation is an issue. We also compare the emission profiles of trucks traveling at low speeds along a level, arterial road en route to the port and at high speeds up a 4% grade highway approaching the tunnel. Given the climate impacts of BC and N2O, we also examine the global warming potential of emissions from trucks with and without DPF and SCR.

HONO and Inorganic Fine Particle Composition in Typical Monsoon Region with Intensive Anthropogenic Emission: In-situ Observations and Source Identification.

Science.gov (United States)

Xie, Y.; Nie, W.; Ding, A.; Huang, X.

2015-12-01

Yangtze River Delta (YRD) is one of the most typical monsoon area with probably the most largest population intensity in the world. With sharply economic development and the large anthropogenic emissions, fine particle pollution have been one of the major air quality problem and may further have impact on the climate system. Though a lot of control policy (sulfur emission have been decreasing from 2007) have been conducted in the region, studies showed the sulfate in fine particles still take major fraction as the nitrate from nitrogen oxides increased significantly. In this study, the role of inorganic chemical compositions in fine particles was investigated with two years in-situ observation. Sulfate and Nitrate contribute to fine particle mass equally in general, but sulfate contributes more during summer and nitrate played more important role in winter. Using lagrangian dispersion backward modeling and source contribution clustering method, the impact of airmass coming from different source region (industrial, dust, biogenic emissions, etc) on fine particle inorganic compositions were discussed. Furthermore, we found two unique cases showing in-situ implications for sulfate formation by nitrogen dioxide oxidation mechanisms. It was showed that the mixing of anthropogenic pollutants with long-range transported mineral dust and biomass burning plume would enhance the sulfate formation by different chemistry mechanisms. This study focus on the complex aspects of fine particle formation in airmasses from different source regions: . It highlights the effect of NOx in enhancing the atmospheric oxidization capacity and indicates a potentially very important impact of increasing NOx on air pollution formation and regional climate change in East Asia.

Upgrading ATLAS Fast Calorimeter Simulation

CERN Document Server

Heath, Matthew Peter; The ATLAS collaboration

2017-01-01

Producing the very large samples of simulated events required by many physics and performance studies with the ATLAS detector using the full GEANT4 detector simulation is highly CPU intensive. Fast simulation tools are a useful way of reducing CPU requirements when detailed detector simulations are not needed. During the LHC Run-1, a fast calorimeter simulation (FastCaloSim) was successfully used in ATLAS. FastCaloSim provides a simulation of the particle energy response at the calorimeter read-out cell level, taking into account the detailed particle shower shapes and the correlations between the energy depositions in the various calorimeter layers. It is interfaced to the standard ATLAS digitization and reconstruction software, and it can be tuned to data more easily than Geant4. Now an improved version of FastCaloSim is in development, incorporating the experience with the version used during Run-1. The new FastCaloSim aims to overcome some limitations of the first version by improving the description of s...

Light particle and gamma ray emission measurements in heavy ion reactions. Progress report

International Nuclear Information System (INIS)

Petitt, G.A.

1983-01-01

Studies of neutron and charged particle emission in heavy ion reactions using the facilities at the HHIRF and the new computer facilities at Georgia State are briefly described. A progress report for 1982 to 1983 is combined with a proposal for work to be performed during 1983 to 1984. Present activities and immediate plans for a run already approved by the Program Advisory Committee of the HHIRF are discussed

Making evident and the analysis of correlations between light particles by means of multidetector INDRA

International Nuclear Information System (INIS)

Gourio, D.

1997-01-01

This thesis reports an light particle interferometric study carried out for the first time by means of an 4π detector. This enabled to extract the proton and deuteron emission time for correctly selected sources. These measurements are extremely worth in the study of hot nuclear matter, particularly for its decaying modes. In this way a clear image of the production chronology of light particles in the heavy ion collision is obtained. In addition, it was possible to make evident the production of fast unstable fragments associated to the decay through pre-equilibrium particles contributing to the very low relative momentum correlation function. This work is the result of a successful event: the association of the 4π INDRA multidetector to the analysis function of the light particle correlation. The real breakthrough achieved by this study was to demonstrate the possibility of full phase space exploration by building the light particle 4 π correlation. In the case of the Xe + Sn system at 45 MeV/u we were able to characterize the collision violence and and to isolate three sources of particle emission. Thus, it was possible to characterize the proton and deuterons emission time for the quasi-target as well as for the quasi-projectile. An important decrease in the characteristic deuteron emission time was observed according as the central collision was approached. Other important results were obtained concerning the proton-proton and proton-deuteron correlation functions as well as the presence of an independent particle dynamical emission of mid-rapidity quasi-targets and quasi- projectiles. Finally, the observation of correlation functions allowed to demonstrate structures at very low relative momentum which can not be understood by the final state interaction only. An explanation could be obtained by a theoretical code taking into account the reaction dynamics, the particle interaction in the final state and the decay of primary excited fragments

IN VIVO EVIDENCE OF FREE RADICAL FORMATION IN THE RAT LUNG AFTER EXPOSURE TO AN EMISSION SOURCE AIR POLLUTION PARTICLE

Science.gov (United States)

Exposure to air pollution particles can be associated with increased human morbidity and mortality. The mechanism(s) of lung injury remains unknown. We tested the hypothesis that lung exposure to oil fly ash (an emission source air pollution particle) causes in vivo free radical ...

Development of a Reference Database for Particle-Induced Gamma-ray Emission spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Dimitriou, P., E-mail: P.Dimitriou@iaea.org [International Atomic Energy Agency, Wagramerstrasse 5, A-1400 Vienna (Austria); Becker, H.-W. [Ruhr Universität Bochum, Gebäude NT05/130, Postfach 102148, Bochum 44721 (Germany); Bogdanović-Radović, I. [Department of Experimental Physics, Institute Rudjer Boskovic, Bijenicka Cesta 54, 10000 Zagreb (Croatia); Chiari, M. [Istituto Nazionale di Fisica Nucleare, Via Sansone 1, Sesto Fiorentino, 50019 Firenze (Italy); Goncharov, A. [Kharkov Institute of Physics and Technology, National Science Center, Akademicheskaya Str.1, Kharkov 61108 (Ukraine); Jesus, A.P. [Departamento de Física, Faculdade de Ciências e Tecnologia da Universidade Nova de Lisboa (Portugal); Kakuee, O. [Nuclear Science and Technology Research Institute, End of North Karegar Ave., PO Box 14395-836, Tehran (Iran, Islamic Republic of); Kiss, A.Z. [Institute of Nuclear Research (ATOMKI), Bem ter 18/c, PO Box 51, 4001 Debrecen (Hungary); Lagoyannis, A. [National Center of Scientific Research “Demokritos”, Agia Paraskevi, P.O. Box 60228, 15310 Athens (Greece); Räisänen, J. [Division of Materials Physics, Department of Physics, University of Helsinki, PO Box 43, 00014 University of Helsinki (Finland); Strivay, D. [Institut de Physique Nucleaire, Atomique et de Spectroscopie, Universite de Liège, Sart Tilman, B15 4000 Liège (Belgium); Zucchiatti, A. [Centro de Micro Análisis de Materiales, Universidad Autónoma de Madrid, Faraday 3, Madrid 28049 (Spain)

2016-03-15

Particle-Induced Gamma-ray Emission (PIGE) is a powerful analytical technique that exploits the interactions of rapid charged particles with nuclei located near a sample surface to determine the composition and structure of the surface regions of solids by measurement of characteristic prompt γ rays. The potential for depth profiling of this technique has long been recognized, however, the implementation has been limited owing to insufficient knowledge of the physical data and lack of suitable user-friendly computer codes for the applications. Although a considerable body of published data exists in the nuclear physics literature for nuclear reaction cross sections with γ rays in the exit channel, there is no up-to-date, comprehensive compilation specifically dedicated to IBA applications. A number of PIGE cross-section data had already been uploaded to the Ion Beam Analysis Nuclear Data Library (IBANDL) ( (http://www-nds.iaea.org/ibandl)) by members of the IBA community by 2011, however a preliminary survey of this body of unevaluated experimental data has revealed numerous discrepancies beyond the uncertainty limits reported by the authors. Using the resources and coordination provided by the IAEA, a concerted effort to improve the situation was made within the Coordinated Research Project on the Development of a Reference Database for PIGE spectroscopy, from 2011 to 2015. The aim of the CRP was to create a data library for Ion Beam Analysis that contains reliable and usable data on charged particle γ-ray emission cross sections that would be made freely available to the user community. As the CRP has reached its completion, we shall present its main achievements, including the results of nuclear cross-section evaluations and the development of a computer code that will become available to the public allowing for the implementation of a standardless PIGE technique.

Experimental investigations of the influence from different operating conditions on the particle emissions from a small-scale pellets combustor

International Nuclear Information System (INIS)

Wiinikka, Henrik; Gebart, Rikard

2004-01-01

The purpose of this study is to determine how different design parameters in an idealised small-scale combustor affect the emission of particulates in the flue gas and to provide insight that can be used for design optimisation. The design parameters are the primary air factor, the total air factor and the magnitude of swirling flow in the combustion chamber. Particles from the reactor were collected from two different sampling lines, one located in the combustion zone, just above the fuel bed, and the other in the flue stack after the reactor. The measurements show that this burner gives very low emissions of particulates and CO in the flue gas. Furthermore, the concentration of particles in the flue gas is uncoupled to the concentration of particles immediately above the fuel bed, probably as a result of a well-designed secondary air supply. The variable that had the strongest effect on the total particulate emission from the combustor was the total air factor. In order to understand the qualitative differences in the flow nature between different operating conditions, CFD simulations of the flow field were also performed

Fast ignition: Dependence of the ignition energy on source and target parameters for particle-in-cell-modelled energy and angular distributions of the fast electrons

Energy Technology Data Exchange (ETDEWEB)

Bellei, C.; Divol, L.; Kemp, A. J.; Key, M. H.; Larson, D. J.; Strozzi, D. J.; Marinak, M. M.; Tabak, M.; Patel, P. K. [Lawrence Livermore National Laboratory, 7000 East Avenue, Livermore, California 94550 (United States)

2013-05-15

The energy and angular distributions of the fast electrons predicted by particle-in-cell (PIC) simulations differ from those historically assumed in ignition designs of the fast ignition scheme. Using a particular 3D PIC calculation, we show how the ignition energy varies as a function of source-fuel distance, source size, and density of the pre-compressed fuel. The large divergence of the electron beam implies that the ignition energy scales with density more weakly than the ρ{sup −2} scaling for an idealized beam [S. Atzeni, Phys. Plasmas 6, 3316 (1999)], for any realistic source that is at some distance from the dense deuterium-tritium fuel. Due to the strong dependence of ignition energy with source-fuel distance, the use of magnetic or electric fields seems essential for the purpose of decreasing the ignition energy.

Light particle emission as a probe of reaction mechanism and nuclear excitation

International Nuclear Information System (INIS)

Guerreau, D.

1989-01-01

The central part of these lectures will be dealing with the problem of energy dissipation. A good understanding of the mechanisms for the dissipation requires to study both peripheral and central collisions or, in other words, to look at the impact paramenter dependence. This should also provide valuable information on the time scale. In order to probe the reaction mechanism and nuclear excitation, one of the most powerful tool is unquestionably the observation of light particle emission, including neutrons and charged particles. Several examples will be discussed related to peripheral collisions (the fate of transfer reactions, the excitation energy generation, the production of projectile-like fragments) as well as inner collisions for which extensive studies have demonstrated the strength of intermediate energy heavy ions for the production of very hot nuclei and detailed study of their decay properties

Measurement of particle emission in automobil exhaust - application of continuous radiometric aerosol measurement to the emission of diesel engines

International Nuclear Information System (INIS)

Krasenbrink, A.; Georgi, B.

1989-01-01

The well-known method of measuring continuously dust by β-absorption is transferred to the problem of particle emission in automobile exhaust. With two similar dust-monitors FH62 having different sampling air flow rates and two low-pressure impactors the reliability of radiometric mass determination was verified. First static experiments with diesel soot showed the necessity of a dilution system, a new mass calibration with regard to the changed β-absorptivity and a quicker calculation of concentration for realtime measurements. (orig.) [de

On the unification of aircraft ultrafine particle emission data

Energy Technology Data Exchange (ETDEWEB)

Kaercher, B.; Busen, R. [DLR Deutsches Zentrum fuer Luft- und Raumfahrt e.V., Wessling (Germany). Inst. fuer Physik der Atmosphaere; Turco, R.P.; Yu Fangqun [California Univ., Los Angeles, CA (United States). Dept. of Atmospheric Sciences; Danilin, M.Y.; Weisenstein, D.K. [Atmospheric and Environmental Research, Inc., Cambridge, MA (United States); Miake-Lye, R.C. [Aerodyne Research, Inc., Billerica, MA (United States)

2000-03-01

To predict the environmental impacts of future commercial aviation, intensive studies have been launched to measure the properties and effects of aircraft emissions. These observations have revealed an extremely wide variance with respect to the number and sizes of the particles produced in the exhaust plumes. Aircraft aerosol ultimately contributes to the population of cloud-forming nuclei, and may lead to significant global radiative and chemical perturbations. In this paper, recent discoveries are coordinated and unified in the form of a physically consistent plume aerosol model that explains most of the observational variance. Using this new approach, it is now practical to carry out reliable global atmospheric simulations of aircraft effects, as demonstrated by a novel assessment of the perturbation of the stratospheric aerosol layer by a supersonic aircraft fleet. (orig.)

Impact of vehicular emissions on the formation of fine particles in the Sao Paulo Metropolitan Area: a numerical study with the WRF-Chem model

Directory of Open Access Journals (Sweden)

A. Vara-Vela

2016-01-01

Full Text Available The objective of this work is to evaluate the impact of vehicular emissions on the formation of fine particles (PM2.5;  ≤  2.5 µm in diameter in the Sao Paulo Metropolitan Area (SPMA in Brazil, where ethanol is used intensively as a fuel in road vehicles. The Weather Research and Forecasting with Chemistry (WRF-Chem model, which simulates feedbacks between meteorological variables and chemical species, is used as a photochemical modelling tool to describe the physico-chemical processes leading to the evolution of number and mass size distribution of particles through gas-to-particle conversion. A vehicular emission model based on statistical information of vehicular activity is applied to simulate vehicular emissions over the studied area. The simulation has been performed for a 1-month period (7 August–6 September 2012 to cover the availability of experimental data from the NUANCE-SPS (Narrowing the Uncertainties on Aerosol and Climate Changes in Sao Paulo State project that aims to characterize emissions of atmospheric aerosols in the SPMA. The availability of experimental measurements of atmospheric aerosols and the application of the WRF-Chem model made it possible to represent some of the most important properties of fine particles in the SPMA such as the mass size distribution and chemical composition, besides allowing us to evaluate its formation potential through the gas-to-particle conversion processes. Results show that the emission of primary gases, mostly from vehicles, led to a production of secondary particles between 20 and 30 % in relation to the total mass concentration of PM2.5 in the downtown SPMA. Each of PM2.5 and primary natural aerosol (dust and sea salt contributed with 40–50 % of the total PM10 (i.e. those  ≤  10 µm in diameter concentration. Over 40 % of the formation of fine particles, by mass, was due to the emission of hydrocarbons, mainly aromatics. Furthermore, an increase in the

Impact of vehicular emissions on the formation of fine particles in the Sao Paulo Metropolitan Area: a numerical study with the WRF-Chem model

Science.gov (United States)

Vara-Vela, A.; Andrade, M. F.; Kumar, P.; Ynoue, R. Y.; Muñoz, A. G.

2016-01-01

The objective of this work is to evaluate the impact of vehicular emissions on the formation of fine particles (PM2.5; ≤ 2.5 µm in diameter) in the Sao Paulo Metropolitan Area (SPMA) in Brazil, where ethanol is used intensively as a fuel in road vehicles. The Weather Research and Forecasting with Chemistry (WRF-Chem) model, which simulates feedbacks between meteorological variables and chemical species, is used as a photochemical modelling tool to describe the physico-chemical processes leading to the evolution of number and mass size distribution of particles through gas-to-particle conversion. A vehicular emission model based on statistical information of vehicular activity is applied to simulate vehicular emissions over the studied area. The simulation has been performed for a 1-month period (7 August-6 September 2012) to cover the availability of experimental data from the NUANCE-SPS (Narrowing the Uncertainties on Aerosol and Climate Changes in Sao Paulo State) project that aims to characterize emissions of atmospheric aerosols in the SPMA. The availability of experimental measurements of atmospheric aerosols and the application of the WRF-Chem model made it possible to represent some of the most important properties of fine particles in the SPMA such as the mass size distribution and chemical composition, besides allowing us to evaluate its formation potential through the gas-to-particle conversion processes. Results show that the emission of primary gases, mostly from vehicles, led to a production of secondary particles between 20 and 30 % in relation to the total mass concentration of PM2.5 in the downtown SPMA. Each of PM2.5 and primary natural aerosol (dust and sea salt) contributed with 40-50 % of the total PM10 (i.e. those ≤ 10 µm in diameter) concentration. Over 40 % of the formation of fine particles, by mass, was due to the emission of hydrocarbons, mainly aromatics. Furthermore, an increase in the number of small particles impaired the

Particle induced X-ray emission for quantitative trace-element analysis using the Eindhoven cyclotron

International Nuclear Information System (INIS)

Kivits, H.

1980-01-01

Development of a multi-elemental trace analysis technique using PIXE (Particle Induced X-ray Emission), was started almost five years ago at the Eindhoven University of Technology, in the Cyclotron Applications Group of the Physics Department. The aim of the work presented is to improve the quantitative aspects of trace-element analysis with PIXE, as well as versatility, speed and simplicity. (Auth.)

Study of luminous emissions associated to electron emissions in radiofrequency cavities; Etude des emissions lumineuses associees aux emissions electroniques dans les cavites hyperfrequences

Energy Technology Data Exchange (ETDEWEB)

Maissa, S

1996-11-26

This study investigates luminous emissions simultaneously to electron emissions and examines their features in order to better understand the field electron emission phenomenon. A RF cavity, operating at room temperature and in pulsed mode, joined to a sophisticated experimental apparatus has been especially developed. The electron and luminous emissions are investigated on cleaned or with metallic, graphitic and dielectric particles contaminated RF surfaces in order to study their influence on these phenomena. During the surface processing, unstable luminous spots glowing during one RF pulse are detected. Their apparition is promoted in the vicinity of the metallic particles or scratches. Two hypotheses could explain their origin: the presence of micro-plasmas associated to electronic explosive emission during processing or the thermal radiation of the melted metal during this emission. Stable luminous spots glowing during several RF pulses are also detected and appear to increase on RF surfaces contaminated with dielectric particles, leading to strong and explosive luminous emissions. Two interpretations are considered: the initiation of surface breakdowns on the dielectric particles or the heating by the RF field at temperatures sufficiently intense to provoke their thermal radiation then their explosion. Finally a superconducting cavity has been adapted to observe luminous spots, which differ from the former ones bu their star shape and could be associated to micro-plasmas, revealed by the starbursts observed on superconducting cavity walls. (author) 102 refs.

Shape of electron lines emitted by a fast particle in atomic collisions. Influence of the acceptance function

International Nuclear Information System (INIS)

Bordenave-Montesquieu, A.; Gleizes, A.; Benoit-Cattin, P.; Boudjema, M.

1980-01-01

In order to explain the large energy broadening of the lines observed in energy spectra of electrons emitted by fast particles, an accurate knowledge of the angular acceptance function of the electron energy analyser is necessary. A simple method is proposed which can give an accurate function for most atomic collisions: the various approximations are discussed. It is also shown that the analyser transmission depends on the acceptance angle. (author)

The quantitative determination of trace elements in giant unicellular plants by particle-induced X-ray emission

International Nuclear Information System (INIS)

Navarrete-Dominguez, V.R.; Yoshihara, K.; Tanaka, N.

1982-01-01

Particle-induced X-ray emission (PIXE) was applied for the determination of trace elements in biologically interesting materials, giant unicellular plants. It was found that the PIXE method had advantages in multi-element trace analysis of a single cell of the sample plant. (author)

Energy spectra and asymmetry of charged particle emission in the muon minus capture by nuclei

International Nuclear Information System (INIS)

Balandin, M.P.; Grebenyuk, V.M.; Sinov, V.G.; Konin, A.D.

1978-01-01

Energy spectra of separated-by-mass single-charged particles at the capture of 130 MeV negative muons by carbon, oxygen, magnesium and sulphur have been measured. The experimental results are compared with the theoretical calculations at the assumption of preequilibrium decay of collective states described by the hydrodynamical model. The measurement of asymmetry of charged particle emission in sulphur and megnesium was carried out by hte method of muon spin precession in a magnetic field. Theoretical curves describe correctly the exponential spectra character, but the yields obtained are 2-3 times less than the experimental results

[Size distribution of particle and polycyclic aromatic hydrocarbons in particle emissions from simulated emission sources].

Science.gov (United States)

Fu, Hai-Huan; Tian, Na; Shang, Hui-Bin; Zhang, Bin; Ye, Su-Fen; Chen, Xiao-Qiu; Wu, Shui-Ping

2014-01-01

Particles from cooking lampblack, biomass and plastics burning smoke, gasoline vehicular exhausts and gasoline generator exhausts were prepared in a resuspension test chamber and collected using a cascade MOUDI impactor. A total of 18 polycyclic aromatic hydrocarbons (PAHs) associated with particles were analyzed by GC-MS. The results showed that there were two peaks in the range of 0.44-1.0 microm and 2.5-10 microm for cooking lampblack, and only one peak in the range of 0.44-1.0 microm for straw and wood burning smoke. But there were no clear peak for plastics burning smoke. The peak for gasoline vehicular exhausts was found in the range of 2.5-10 microm due to the influence of water vapor associated with particles, while the particles from gasoline generator exhausts were mainly in the range of lampblack and gasoline vehicular exhausts. The peak in the range of 0.44-1.0 microm became more and more apparent with the increase of PAHs molecular weight. The fraction of PAH on particles less than 1.0 microm to that on the total particles increased along with PAH's molecular weight. Phenanthrene was the dominant compound for cooking lampblack and combustion smoke, while gasoline vehicular exhausts and generator exhausts were characterized with significantly high levels of naphthalene and benzo[g, h, i] perylene, respectively. The distribution of source characteristic ratios indicated that PAHs from cooking lampblack and biomass burning were close and they were different from those of vehicular exhausts and generator exhausts.

Fast particle tracking with wake fields

Energy Technology Data Exchange (ETDEWEB)

Dohlus, M.; Floettmann, K.; Henning, C.

2012-01-15

Tracking calculations of charged particles in electromagnetic fields require in principle the simultaneous solution of the equation of motion and of Maxwell's equations. In many tracking codes a simpler and more efficient approach is used: external fields like that of the accelerating structures are provided as field maps, generated in separate computations and for the calculation of self fields the model of a particle bunch in uniform motion is used. We describe how an externally computed wake function can be approximated by a table of Taylor coefficients and how the wake field kick can be calculated for the particle distribution in a tracking calculation. The integrated kick, representing the effect of a distributed structure, is applied at a discrete time. As an example, we use our approach to calculate the emittance growth of a bunch in an undulator beam pipe due to resistive wall wake field effects. (orig.)

Components of Particle Emissions from Light-Duty Spark-Ignition Vehicles with Varying Aromatic Content and Octane Rating in Gasoline.

Science.gov (United States)

Short, Daniel Z; Vu, Diep; Durbin, Thomas D; Karavalakis, Georgios; Asa-Awuku, Akua

2015-09-01

Typical gasoline consists of varying concentrations of aromatic hydrocarbons and octane ratings. However, their impacts on particulate matter (PM) such as black carbon (BC) and water-soluble and insoluble particle compositions are not well-defined. This study tests seven 2012 model year vehicles, which include one port fuel injection (PFI) configured hybrid vehicle, one PFI vehicle, and six gasoline direct injection (GDI) vehicles. Each vehicle was driven on the Unified transient testing cycle (UC) using four different fuels. Three fuels had a constant octane rating of 87 with varied aromatic concentrations at 15%, 25%, and 35%. A fourth fuel with higher octane rating, 91, contained 35% aromatics. BC, PM mass, surface tension, and water-soluble organic mass (WSOM) fractions were measured. The water-insoluble mass (WIM) fraction of the vehicle emissions was estimated. Increasing fuel aromatic content increases BC emission factors (EFs) of transient cycles. BC concentrations were higher for the GDI vehicles than the PFI and hybrid vehicles, suggesting a potential climate impact for increased GDI vehicle production. Vehicle steady-state testing showed that the hygroscopicity of PM emissions at high speeds (70 mph; κ > 1) are much larger than emissions at low speeds (30 mph; κ < 0.1). Iso-paraffin content in the fuels was correlated to the decrease in WSOM emissions. Both aromatic content and vehicle speed increase the amount of hygroscopic material found in particle emissions.

FAST, LOW-IONIZATION EMISSION REGIONS OF THE PLANETARY NEBULA M2-42

Energy Technology Data Exchange (ETDEWEB)

Danehkar, A.; Parker, Q. A. [Department of Physics and Astronomy, Macquarie University, Sydney, NSW 2109 (Australia); Steffen, W., E-mail: ashkbiz.danehkar@cfa.harvard.edu [Instituto de Astronomía, Universidad Nacional Autónoma de México, C.P.22860, Ensenada (Mexico)

2016-02-15

Spatially resolved observations of the planetary nebula M2-42 (PN G008.2−04.8) obtained with the Wide Field Spectrograph on the Australian National University 2.3 m telescope have revealed the remarkable features of bipolar collimated jets emerging from its main structure. Velocity-resolved channel maps derived from the [N ii] λ6584 emission line disentangle different morphological components of the nebula. This information is used to develop a three-dimensional morpho-kinematic model, which consists of an equatorial dense torus and a pair of asymmetric bipolar outflows. The expansion velocity of about 20 km s{sup −1} is measured from the spectrum integrated over the main shell. However, the deprojected velocities of the jets are found to be in the range of 80–160 km s{sup −1} with respect to the nebular center. It is found that the mean density of the collimated outflows, 595 ± 125 cm{sup −3}, is five times lower than that of the main shell, 3150 cm{sup −3}, whereas their singly ionized nitrogen and sulfur abundances are about three times higher than those determined from the dense shell. The results indicate that the features of the collimated jets are typical of fast, low-ionization emission regions.

PEPT: An invaluable tool for 3-D particle tracking and CFD simulation verification in hydrocyclone studies

Directory of Open Access Journals (Sweden)

Hoffmann Alex C.

2013-05-01

Full Text Available Particle tracks in a hydrocyclone generated both experimentally by positron emission particle tracking (PEPT and numerically with Eulerian-Lagranian CFD have been studied and compared. A hydrocyclone with a cylinder-on-cone design was used in this study, the geometries used in the CFD simulations and in the experiments being identical. It is shown that it is possible to track a fast-moving particle in a hydrocyclone using PEPT with high temporal and spatial resolutions. The numerical 3-D particle trajectories were generated using the Large Eddy Simulation (LES turbulence model for the fluid and Lagrangian particle tracking for the particles. The behaviors of the particles were analyzed in detail and were found to be consistent between experiments and CFD simulations. The tracks of the particles are discussed and related to the fluid flow field visualized in the CFD simulations using the cross-sectional static pressure distribution.

Effects of fibre-form nanostructures on particle emissions from a tungsten surface in plasmas

International Nuclear Information System (INIS)

Takamura, S.; Miyamoto, T.; Ohno, N.

2012-01-01

The effects of fibre-form nanostructure of a tungsten surface on both electron emission and sputtering in helium/argon plasmas are represented. Generally, a nano-fibre forest, the so-called ‘fuzz’, made of tungsten with helium gas inside is found to have the tendency of suppressing the particle emission substantially. The electron emission comes from the impact of high-energy primary electrons. In addition, a deeply biased tungsten target, which inhibits the influx of even energetic primary electrons, seems to produce an electron emission, and it may be suppressed on the way to nanostructure formation on the surface of the W target. Such an emission process is discussed here. The sputtering yield of the He-damaged tungsten surface with the fibre-form nanostructure depends on the surface morphology while the sputtering itself changes the surface morphology, so that the time evolutions of sputtering yield from the W surface with an originally well-developed nanostructure are found to show a minimum in sputtering yield, which is about a half for the fresh nanostructured tungsten and roughly one-fifth of the yield for the original flat normal tungsten surface. The surface morphology at that time is, for the first time, made clear with field emission scanning electron microscopy observation. The physical mechanism for the appearance of such a minimum in sputtering yield is discussed. (paper)

Soot, unburned carbon and ultrafine particle emissions from air- and oxy-coal flames

International Nuclear Information System (INIS)

Morris, W.J.; Yu, Dunxi; Wendt, J.O.L.

2010-01-01

Oxy-coal combustion is one possible solution for the mitigation of greenhouse gases. In this process coal is burned in oxygen, rather than air, and the temperatures in the boiler are mitigated by recycling flue gases, so that the inlet mixture may contain either 27 % O 2 to match adiabatic flame temperatures, or 32 % O 2 to match gaseous radiation heat fluxes in the combustion chamber. However, a major issue for heat transfer from coal combustion is the radiative heat transmission from soot. For this research, air and oxy coal firing were compared regarding the emission of soot. A 100 kW down-fired laboratory combustor was used to determine effects of switching from air to oxy-firing on soot, unburned carbon and ultrafine particle emissions from practical pulverized coal flames. Of interest here were potential chemical effects of substitution of the N 2 in air by CO 2 in practical pulverized coal flames. The oxy-coal configuration investigated used once-through CO 2 , simulating cleaned flue gas recycle with all contaminants and water removed. Three coals were each burned in: a) air, b) 27 % O 2 / 73 % CO 2 , c) 32 % O 2 / 68 % CO 2 . Tests were conducted at (nominally) 3 %, 2 %, 1 % and 0 % O 2 in the exhaust (dry basis). For each condition, particulate samples were iso kinetically withdrawn far from the radiant zone, and analyzed using a photoacoustic analyzer (PA) for black carbon, a scanning mobility particle sizer (SMPS) for ultrafine particles, and a total sample loss on ignition (LOI) method for unburned carbon in ash. Data suggest that at low stoichiometric ratios, ultrafine particles consist primarily of black carbon, which, for the bituminous coal, is produced in lesser amounts under oxy-fired conditions than under the air-fired condition, even when adiabatic flame temperatures are matched. However, significant changes in mineral matter vaporization were not observed unless the flames were hotter. These and other results are interpreted in the light of

Total Particle Number Emissions from Modern Diesel, Natural Gas, and Hybrid Heavy-Duty Vehicles During On-Road Operation.

Science.gov (United States)

Wang, Tianyang; Quiros, David C; Thiruvengadam, Arvind; Pradhan, Saroj; Hu, Shaohua; Huai, Tao; Lee, Eon S; Zhu, Yifang

2017-06-20

Particle emissions from heavy-duty vehicles (HDVs) have significant environmental and public health impacts. This study measured total particle number emission factors (PNEFs) from six newly certified HDVs powered by diesel and compressed natural gas totaling over 6800 miles of on-road operation in California. Distance-, fuel- and work-based PNEFs were calculated for each vehicle. Distance-based PNEFs of vehicles equipped with original equipment manufacturer (OEM) diesel particulate filters (DPFs) in this study have decreased by 355-3200 times compared to a previous retrofit DPF dynamometer study. Fuel-based PNEFs were consistent with previous studies measuring plume exhaust in the ambient air. Meanwhile, on-road PNEF shows route and technology dependence. For vehicles with OEM DPFs and Selective Catalytic Reduction Systems, PNEFs under highway driving (i.e., 3.34 × 10 12 to 2.29 × 10 13 particles/mile) were larger than those measured on urban and drayage routes (i.e., 5.06 × 10 11 to 1.31 × 10 13 particles/mile). This is likely because a significant amount of nucleation mode volatile particles were formed when the DPF outlet temperature reached a critical value, usually over 310 °C, which was commonly achieved when vehicle speed sustained over 45 mph. A model year 2013 diesel HDV produced approximately 10 times higher PNEFs during DPF active regeneration events than nonactive regeneration.

Numerical Simulation to Phenomenon of Main Vessel Free Surface Flow Impact Coping for Fast Reactor by Moving Particle Semi-implicit Method

International Nuclear Information System (INIS)

Wei Yuanyuan; Lu Daogang

2009-01-01

There is the free surface in the main vessel of fast reactor, when long period earthquakes happen, the fluid will impact the coping of vessel and make the reactor dangerous. The flow of the fluid was simulated by moving particle semi-implicit method. The phenomenon on sloshing response of the free surface in the main vessel of fast reactor excited by 3 sine waves was simulated. The impact pressure from the research can provide important loadings for the integrality analysis of the main vessel. (authors)

Impacts of Mid-level Biofuel Content in Gasoline on SIDI Engine-Out and Tailpipe Particulate Matter Emissions: Preprint

Energy Technology Data Exchange (ETDEWEB)

He, X.; Ireland, J. C.; Zigler, B. T.; Ratcliff, M. A.; Knoll, K. E.; Alleman, T. L.; Tester, J. T.

2011-02-01

The influences of ethanol and iso-butanol blended with gasoline on engine-out and post Three-Way Catalyst (TWC) particle size distribution and number concentration were studied using a GM 2.0L turbocharged Spark Ignition Direct Injection (SIDI) engine. The engine was operated using the production ECU with a dynamometer controlling the engine speed and the accelerator pedal position controlling the engine load. A TSI Fast Mobility Particle Sizer (FMPS) spectrometer was used to measure the particle size distribution in the range from 5.6 to 560 nm with a sampling rate of 1 Hz. US federal certification gasoline (E0), two ethanol-blended fuels (E10 and E20), and 11.7% iso-butanol blended fuel (BU12) were tested. Measurements were conducted at ten selected steady-state engine operation conditions. Bi-modal particle size distributions were observed for all operating conditions with peak values at particle sizes of 10 nm and 70 nm. Idle and low speed / low load conditions emitted higher total particle numbers than other operating conditions. At idle, the engine-out Particulate Matter (PM) emissions were dominated by nucleation mode particles, and the production TWC reduced these nucleation mode particles by more than 50%, while leaving the accumulation mode particle distribution unchanged. At engine load higher than 6 bar NMEP, accumulation mode particles dominated the engine-out particle emissions and the TWC had little effect. Compared to the baseline gasoline (E0), E10 does not significantly change PM emissions, while E20 and BU12 both reduce PM emissions under the conditions studied. Iso-butanol was observed to impact PM emissions more than ethanol, with up to 50% reductions at some conditions. In this paper, the issues related to PM measurement using FMPS are also discussed. While some uncertainties are due to engine variation, the FMPS must be operated under careful maintenance procedures in order to achieve repeatable measurement results.

Fast Calorimeter Simulation in ATLAS

CERN Document Server

Schaarschmidt, Jana; The ATLAS collaboration

2017-01-01

Producing the very large samples of simulated events required by many physics and performance studies with the ATLAS detector using the full GEANT4 detector simulation is highly CPU intensive. Fast simulation tools are a useful way of reducing CPU requirements when detailed detector simulations are not needed. During the LHC Run-1, a fast calorimeter simulation (FastCaloSim) was successfully used in ATLAS. FastCaloSim provides a simulation of the particle energy response at the calorimeter read-out cell level, taking into account the detailed particle shower shapes and the correlations between the energy depositions in the various calorimeter layers. It is interfaced to the standard ATLAS digitization and reconstruction software, and it can be tuned to data more easily than GEANT4. It is 500 times faster than full simulation in the calorimeter system. Now an improved version of FastCaloSim is in development, incorporating the experience with the version used during Run-1. The new FastCaloSim makes use of mach...

Design of a Fast Neutral He Beam System for Feasibility Study of Charge-Exchange Alpha-Particle Diagnostics in a Thermonuclear Fusion Reactor

CERN Document Server

Shinto, Katsuhiro; Kitajima, Sumio; Kiyama, Satoru; Nishiura, Masaki; Sasao, Mamiko; Sugawara, Hiroshi; Takenaga, Mahoko; Takeuchi, Shu; Wada, Motoi

2005-01-01

For alpha-particle diagnostics in a thermonuclear fusion reactor, neutralization using a fast (~2 MeV) neutral He beam produced by the spontaneous electron detachment of a He- is considered most promising. However, the beam transport of produced fast neutral He has not been studied, because of difficulty for producing high-brightness He- beam. Double-charge-exchange He- sources and simple beam transport systems were developed and their results were reported in the PAC99* and other papers.** To accelerate an intense He- beam and verify the production of the fast neutral He beam, a new test stand has been designed. It consists of a multi-cusp He+

Emission of Gas and Al2O3 Smoke in Gas-Al Particle Deflagration: Experiments and Emission Modeling for Explosive Fireballs

Science.gov (United States)

Ranc-Darbord, Isabelle; Baudin, Gérard; Genetier, Marc; Ramel, David; Vasseur, Pierre; Legrand, Julien; Pina, Vincent

2018-03-01

Emission of gas and Al2O3 smoke within the deflagration of H2{-}O2-{N2{-}CO2}-Al particles has been studied in a closed combustion chamber at pressures of up to 18 bar and at gas temperatures of up to 3700 K. Measurements of radiance intensity were taken using a five wavelength pyrometer (0.660 μ m, 0.850 μ m, 1.083 μ m, 1.260 μ m, 1.481 μ m) and a grating spectrometer in the range (4.10 μ m to 4.30 μ m). In order to characterize the aluminum oxide smoke size and temperature, an inversion method has been developed based on the radiation transfer equation and using pyrometer measurements and thermochemical calculations of Al2O3 smoke volume fractions. Temperatures in combustion gas have been determined using a method based on the assumed blackbody head of the 4.26 μ m CO2 emission line and on its spectral shift with pressure and temperature. For validation purpose, this method has been applied to measurements obtained when calibrated alumina particles are injected in a combustion chamber prior to gaseous deflagrations. This mathematical inversion method was developed to investigate explosive fireballs.

Reduced Ultrafine Particle Concentration in Urban Air: Changes in Nucleation and Anthropogenic Emissions.

Science.gov (United States)

Saha, Provat K; Robinson, Ellis S; Shah, Rishabh U; Zimmerman, Naomi; Apte, Joshua S; Robinson, Allen L; Presto, Albert A

2018-06-19

Nucleation is an important source of ambient ultrafine particles (UFP). We present observational evidence of the changes in the frequency and intensity of nucleation events in urban air by analyzing long-term particle size distribution measurements at an urban background site in Pittsburgh, Pennsylvania during 2001-2002 and 2016-2017. We find that both frequency and intensity of nucleation events have been reduced by 40-50% over the past 15 years, resulting in a 70% reduction in UFP concentrations from nucleation. On average, the particle growth rates are 30% slower than 15 years ago. We attribute these changes to dramatic reductions in SO 2 (more than 90%) and other pollutant concentrations. Overall, UFP concentrations in Pittsburgh have been reduced by ∼48% in the past 15 years, with a ∼70% reduction in nucleation, ∼27% in weekday local sources (e.g., weekday traffic), and 49% in the regional background. Our results highlight that a reduction in anthropogenic emissions can considerably reduce nucleation events and UFP concentrations in a polluted urban environment.

Aerosol vertical distribution, new particle formation, and jet aircraft particle emissions in the free troposhere and tropopause region; Vertikalverteilung und Neubildungsprozesse des Aerosols und partikelfoermige Flugzeugemissionen in der freien Troposphaere und Tropopausenregion

Energy Technology Data Exchange (ETDEWEB)

Schroeder, F P

2000-07-01

A contribution to the understanding of natural and anthropogenously induced particle formation as well as aerosol physical transformation processes within the free troposphere (FT) is introduced. Documentation and interpretation of empirical data relevant with respect to possible climatologic impact of anthropogenous aerosol emissions into the atmosphere is presented. The first section describes new technique for high spatial resolution measurements of ultrafine aerosol particles by condensation nucleus counters (CNCs), a necessary prerequisite for the observation of natural particle formation and jet aircraft emissions. The second section illustrates vertical distribution and variability ranges of the aerosol in the FT and the tropopause region (TP). Typical microphysical states of the atmospheric aerosol within the Northern Hemisphere are documented by means of systematic measurements during more than 60 flight missions. Simple mathematical parameterizations of the aerosol vertical distribution and aerosol size distributions are developed. Important aerosol sources within the FT are localized and possible aerosol formation processes are discussed. The third section is focussed on jet-engine particle emissions within the FT and TP. A unique inflight experiment for detection of extremely high concentrations (>10{sup 6} cm{sup -3}) of extremely small (donw to <3 nm) aerosols inside the exhaust plumes of several jet aircraft is described. Particle emission indices and emission-controlling parameters are deduced. Most important topic is the impact of fuel sulfur content of kerosine on number, size and chemical composition of jet particle emissions. Generalized results are parameterized in form of lognormal aerosol particle size distributions. (orig.) [German] Ein Beitrag zum Verstaendnis natuerlicher und anthropogen induzierter Aerosolneubildung sowie physikalischer Aerosolumwandlung in der freien Troposphaere wird vorgestellt. Empirisch gewonnenes Datenmaterial wird

Reducing field emission in the superconducting rf cavities for the next generation of particle accelerators

International Nuclear Information System (INIS)

Shu, Q.S.; Hartung, W.; Leibovich, A.; Kirchgessner, J.; Moffat, D.; Padamsee, H.; Rubin, D.; Sears, J.

1991-01-01

This paper reports on field emission, which is an obstacle to reaching the higher fields called for in future applications of superconducting radio frequency cavities to particle accelerators. The authors used heat treatment up to 1500 degrees C in an ultra-high vacuum furnace, along with processing of cavities and temperature mapping, to suppress field emission and analyze emitter properties. In 27 tests of 1-cell 1500 MHz fired accelerating cavities, on the average the accelerating field E acc increased to 24 MV/m (H pk = 1250 Oe) from 13 MV/m with chemical treatment alone; the highest E acc reached was 30.5 MV/m

The new ATLAS Fast Calorimeter Simulation

CERN Document Server

Hasib, Ahmed; The ATLAS collaboration

2017-01-01

Producing the very large samples of simulated events required by many physics and performance studies with the ATLAS detector using the full GEANT4 detector simulation is highly CPU intensive. Fast simulation tools are a useful way of reducing CPU requirements when detailed detector simulations are not needed. During the LHC Run-1, a fast calorimeter simulation (FastCaloSim) was successfully used in ATLAS. FastCaloSim provides a simulation of the particle energy response at the calorimeter read-out cell level, taking into account the detailed particle shower shapes and the correlations between the energy depositions in the various calorimeter layers. It is interfaced to the standard ATLAS digitization and reconstruction software, and it can be tuned to data more easily than GEANT4. Now an improved version of FastCaloSim is in development, incorporating the experience with the version used during Run-1. The new FastCaloSim makes use of statistical techniques such as principal component analysis, and a neural n...

The New ATLAS Fast Calorimeter Simulation

CERN Document Server

Heath, Matthew Peter; The ATLAS collaboration

2017-01-01

Producing the large samples of simulated events required by many physics and performance studies with the ATLAS detector using the full GEANT4 detector simulation is highly CPU intensive. Fast simulation tools are a useful way of reducing the CPU requirements when detailed detector simulations are not needed. During Run-1 of the LHC, a fast calorimeter simulation (FastCaloSim) was successfully used in ATLAS. FastCaloSim provides a simulation of the particle energy response at the calorimeter read-out cell level, taking into account the detailed particle shower shapes and the correlations between the energy depositions in the various calorimeter layers. It is interfaced to the standard ATLAS digitisation and reconstruction software, and it can be tuned to data more easily than Geant4. Now an improved version of FastCaloSim is in development, incorporating the experience with the version used during Run-1. The new FastCaloSim aims to overcome some limitations of the first version by improving the description of...

Pre-equilibrium gamma emissions

International Nuclear Information System (INIS)

Ghosh, Sudip

1993-01-01

Together with the direct reaction and the compound nuclear emissions the pre-equilibrium (PEQ) or pre-compound processes give a fairly complete picture of nuclear reactions induced by light ions at energies of some tens of MeV. PEQ particle emissions covering the higher energy continuum spectra have been investigated in detail both experimentally and theoretically. In contrast, very little work has been done on PEQ γ- emissions. The reason is that in spite of extensive work done on PEQ particle emissions, the mechanism is not yet fully understood. Also, the PEQ γ-emission cross-sections (∼ micro barns) are very small compared to the PEQ particle emission cross-sections (∼ milli barns). Yet apart from the academic interest the understanding of PEQ γ-emissions is important for applied fusion research etc. In this paper the PEQ γ-emissions is discussed and the work done in this field is reviewed. (author). 14 refs