Quinary excitation method for pulse compression ultrasound measurements.

Science.gov (United States)

Cowell, D M J; Freear, S

2008-04-01

A novel switched excitation method for linear frequency modulated excitation of ultrasonic transducers in pulse compression systems is presented that is simple to realise, yet provides reduced signal sidelobes at the output of the matched filter compared to bipolar pseudo-chirp excitation. Pulse compression signal sidelobes are reduced through the use of simple amplitude tapering at the beginning and end of the excitation duration. Amplitude tapering using switched excitation is realised through the use of intermediate voltage switching levels, half that of the main excitation voltages. In total five excitation voltages are used creating a quinary excitation system. The absence of analogue signal generation and power amplifiers renders the excitation method attractive for applications with requirements such as a high channel count or low cost per channel. A systematic study of switched linear frequency modulated excitation methods with simulated and laboratory based experimental verification is presented for 2.25 MHz non-destructive testing immersion transducers. The signal to sidelobe noise level of compressed waveforms generated using quinary and bipolar pseudo-chirp excitation are investigated for transmission through a 0.5m water and kaolin slurry channel. Quinary linear frequency modulated excitation consistently reduces signal sidelobe power compared to bipolar excitation methods. Experimental results for transmission between two 2.25 MHz transducers separated by a 0.5m channel of water and 5% kaolin suspension shows improvements in signal to sidelobe noise power in the order of 7-8 dB. The reported quinary switched method for linear frequency modulated excitation provides improved performance compared to pseudo-chirp excitation without the need for high performance excitation amplifiers.

Process and device for the selective excitation and separation of isotopes

International Nuclear Information System (INIS)

Ducas, T.W.

1976-01-01

Description is given of a method for selectively populating high-lying excited states of atoms or molecules. It comprises: excitation of atoms or molecules with a first circularly polarized pulsed radiation, the coherent frequency components of first pulsed radiation have frequencies corresponding to the energy difference between a lower energy level and the frequency split levels of an intermediate energy level, the duration of pulse being less than 2π/Δω, where Δω is the frequency difference of the split levels; applying a second circularly polarized pulsed radiation to atoms or molecules for a time subsequent to the termination of first radiation, the coherent frequency components of second pulsed radiation have frequencies corresponding to the energy difference between the split levels of intermediate energy level and an upper energy level, the duration of second pulse being less than 2π/Δω. The first and second radiation have the same handedness of circular polarization, whereby upper energy level has a greater population than prior to excitation by first and second radiation pulses [fr

Direct electron-impact mechanism of excitation of mercury monobromide in a double-pulse dielectric-barrier-discharge HgBr lamp

Science.gov (United States)

Datsyuk, V. V.; Izmailov, I. A.; Naumov, V. V.; Kochelap, V. A.

2016-08-01

In a nonequlibrium plasma of a gas-discharge HgBr lamp, the terminal electronic state of the HgBr(B-X) radiative transition with a peak wavelength of 502 nm remains populated for a relatively long time and is repeatedly excited to the B state in collisions with plasma electrons. This transfer of the HgBr molecules from the ground state X to the excited state B is the main mechanism of formation of the light-emitting molecules especially when the lamp is excited by double current pulses. According to our simulations, due to the electron-induced transitions between HgBr(X) and HgBr(B), the output characteristics of the DBD lamp operating in a double-pulse regime are better than those of the lamp operating in a single-pulse regime. In the considered case, the peak power is calculated to increase by a factor of about 2 and the lamp efficiency increases by about 50%.

Experimental installation for excitation of semiconductors and dielectrics by picosecond pulsed electron beam and electric field

International Nuclear Information System (INIS)

Nasibov, A.S.; Berezhnoj, K.V.; Shapkin, P.V.; Reutova, A.G.; Shunajlov, S.A.; Yalandin, M.I.

2009-01-01

The experimental facility for shaping high-voltage pulses with amplitudes of 30-250 kV and durations of 100-500 ps and electron beams with a current density of up to 1000 A/cm -2 is described. The facility was built using the principle of energy compression of a pulse from a nanosecond high-voltage generator accompanied by the subsequent pulse sharpening and cutting. The setup is equipped with two test coaxial chambers for radiation excitation in semiconductor crystals by an electron beam or an electric field in air at atmospheric pressure and T = 300 K. Generation of laser radiation in the visible range under field and electron pumping was attained in ZnSSe, ZnSe, ZnCdS, and CdS (462, 480, 515, and 525 nm, respectively). Under the exposure to an electric field (up to 10 6 V x cm -1 ), the laser generation region is as large as 300-500 μm. The radiation divergence was within 5 Deg C. The maximum integral radiation power (6 kW at λ = 480 nm) was obtained under field pumping of a zinc selenide sample with a single dielectric mirror [ru

Pulsed excitation terahertz tomography - multiparametric approach

Science.gov (United States)

Lopato, Przemyslaw

2018-04-01

This article deals with pulsed excitation terahertz computed tomography (THz CT). Opposite to x-ray CT, where just a single value (pixel) is obtained, in case of pulsed THz CT the time signal is acquired for each position. Recorded waveform can be parametrized - many features carrying various information about examined structure can be calculated. Based on this, multiparametric reconstruction algorithm was proposed: inverse Radon transform based reconstruction is applied for each parameter and then fusion of results is utilized. Performance of the proposed imaging scheme was experimentally verified using dielectric phantoms.

Heat pulse excitability of vestibular hair cells and afferent neurons.

Science.gov (United States)

Rabbitt, Richard D; Brichta, Alan M; Tabatabaee, Hessam; Boutros, Peter J; Ahn, JoongHo; Della Santina, Charles C; Poppi, Lauren A; Lim, Rebecca

2016-08-01

In the present study we combined electrophysiology with optical heat pulse stimuli to examine thermodynamics of membrane electrical excitability in mammalian vestibular hair cells and afferent neurons. We recorded whole cell currents in mammalian type II vestibular hair cells using an excised preparation (mouse) and action potentials (APs) in afferent neurons in vivo (chinchilla) in response to optical heat pulses applied to the crista (ΔT ≈ 0.25°C per pulse). Afferent spike trains evoked by heat pulse stimuli were diverse and included asynchronous inhibition, asynchronous excitation, and/or phase-locked APs synchronized to each infrared heat pulse. Thermal responses of membrane currents responsible for APs in ganglion neurons were strictly excitatory, with Q10 ≈ 2. In contrast, hair cells responded with a mix of excitatory and inhibitory currents. Excitatory hair cell membrane currents included a thermoelectric capacitive current proportional to the rate of temperature rise (dT/dt) and an inward conduction current driven by ΔT An iberiotoxin-sensitive inhibitory conduction current was also evoked by ΔT, rising in protein biophysics and manipulate cellular excitability. Copyright © 2016 the American Physiological Society.

Excitation of nuclear states by synchrotron radiation

International Nuclear Information System (INIS)

Olariu, Albert

2003-01-01

We study the excitation of nuclear states by gamma ray beams of energy up to 200 keV produced as synchrotron radiation. We consider the possibility to populate an excited state |i> in two steps, from the ground state |g> to an intermediary state |n> which decays by gamma emission or internal conversion to a lower state |i>. The aim of this study is to establish that the probability P 2 of the two-step transition |g> → |n> → |i> should be greater than the probability P 1 of the direct transition |g> → |i>. The probabilities P 1 and P 2 correspond to a radiation pulse of duration equal to the half-time of the state |i>. We have written a computer program in C++ which computes the probability P 2 , the ratio P 2 /P 1 and the rate C 2 of the two-step transitions for any nuclei and different configurations of states. The program uses a database which contains information on the energy levels, half-lives, spins and parities of nuclear states and on the relative intensities of the nuclear transitions. If the half-lives or the relative intensities are not known the program uses the Weisskopf estimates for the transition half-lives. An interpolation program of internal conversion coefficients has also been used. We listed the values obtained for P 2 , P 2 /P 1 and C 2 in a number of cases in which P 2 is significant from the 2900 considered cases. The states |i> and |n> have the energies E i and E n , the corresponding half-lives being t i and t n . The spectral density of the synchrotron radiation has been considered to be 10 12 photons cm -2 s -1 eV -1 . We listed only the cases for which the relative intensities of the transitions from levels |n> and |i> to lower states are known. The calculations carried out in this study allowed us to identify nuclei for which P 2 has relatively great values. In the listed cases P 2 /P 1 >>1, so that the two-step excitation by synchrotron radiation is more efficient than the direct excitation |g> → |i>. For a sample having 10

Broadband excitation by chirped pulses: application to single electron spins in diamond

International Nuclear Information System (INIS)

Niemeyer, I; Shim, J H; Zhang, J; Suter, D; Taniguchi, T; Teraji, T; Abe, H; Onoda, S; Yamamoto, T; Ohshima, T; Isoya, J; Jelezko, F

2013-01-01

Pulsed excitation of broad spectra requires very high field strengths if monochromatic pulses are used. If the corresponding high power is not available or not desirable, the pulses can be replaced by suitable low-power pulses that distribute the power over a wider bandwidth. As a simple case, we use microwave pulses with a linear frequency chirp. We use these pulses to excite spectra of single nitrogen–vacancy centres in a Ramsey experiment. Compared to the conventional Ramsey experiment, our approach increases the bandwidth by at least an order of magnitude. Compared to the conventional continuous wave-ODMR experiment, the chirped Ramsey experiment does not suffer from power broadening and increases the resolution by at least an order of magnitude. As an additional benefit, the chirped Ramsey spectrum contains not only ‘allowed’ single quantum transitions, but also ‘forbidden’ zero- and double quantum transitions, which can be distinguished from the single quantum transitions by phase-shifting the readout pulse with respect to the excitation pulse or by variation of the external magnetic field strength. (paper)

Ultrashort-pulse-train pump and dump excitation of a diatomic molecule

Science.gov (United States)

de Araujo, Luís E. E.

2010-09-01

An excitation scheme is proposed for transferring population between ground-vibrational levels of a molecule. The transfer is accomplished by pumping and dumping population with a pair of coherent ultrashort-pulse trains via a stationary state. By mismatching the teeth of the frequency combs associated with the pulse trains to the vibrational levels, high selectivity in the excitation, along with high transfer efficiency, is predicted. The pump-dump scheme does not suffer from spontaneous emission losses, it is insensitive to the pump-dump-train delay, and it requires only basic pulse shaping.

Ultrafast emission from colloidal nanocrystals under pulsed X-ray excitation

CERN Document Server

Turtos, R.M.; Polovitsyn, A.; Christodoulou, S.; Salomoni, M.; Auffray, E.; Moreels, I.; Lecoq, P.; Grim, J.Q.

2016-01-01

Fast timing has emerged as a critical requirement for radiation detection in medical and high energy physics, motivating the search for scintillator materials with high light yield and fast time response. However, light emission rates from conventional scintillation mechanisms fundamentally limit the achievable time resolution, which is presently at least one order of magnitude slower than required for next-generation detectors. One solution to this challenge is to generate an intense prompt signal in response to ionizing radiation. In this paper, we present colloidal semiconductor nanocrystals (NCs) as promising prompt photon sources. We investigate two classes of NCs: two-dimensional CdSe nanoplatelets (NPLs) and spherical CdSe/CdS core/giant shell quantum dots (GS QDs). We demonstrate that the emission rates of these NCs under pulsed X-ray excitation are much faster than traditional mechanisms in bulk scintillators, i.e. 5d-4f transitions. CdSe NPLs have a sub-100 ps effective decay time of 77 ps and CdSe/...

Clinical Comparison of Pulse and Chirp Excitation

DEFF Research Database (Denmark)

Pedersen, Morten Høgholm; Misaridis, T.; Jensen, Jørgen Arendt

2002-01-01

Coded excitation (CE) using frequency modulated signals (chirps) combined with modified matched filtering has earlier been presented showing promising results in simulations and in-vitro. In this study an experimental ultrasound system is evaluated in a clinical setting, where image sequences...... and short pulse excitation to simultaneously produce identical image sequences using both techniques. Nine healthy male volunteers were scanned in abdominal locations. All sequences were evaluated by 3 skilled medical doctors, blinded to each other and to the technique used. They assessed the depth (1...

Multiple pulse traveling wave excitation of neon-like germanium

International Nuclear Information System (INIS)

Moreno, J. C.; Nilsen, J.; Silva, L. B. da

1995-01-01

Traveling wave excitation has been shown to significantly increase the output intensity of the neon-like germanium x-ray laser. The driving laser pulse consisted of three 100 ps Gaussian laser pulses separated by 400 ps. Traveling wave excitation was employed by tilting the wave front of the driving laser by 45 degrees to match the propagation speed of the x-ray laser photons along the length of the target. We show results of experiments with the traveling wave, with no traveling wave, and against the traveling wave and comparisons to a numerical model. Gain was inferred from line intensity measurements at two lengths

Sources of pulsed radiation

International Nuclear Information System (INIS)

Sauer, M.C. Jr.

1981-01-01

Characteristics of various sources of pulsed radiation are examined from the viewpoint of their importance to the radiation chemist, and some examples of uses of such sources are mentioned. A summary is given of the application of methods of physical dosimetry to pulsed sources, and the calibration of convenient chemical dosimeters by physical dosimetry is outlined. 7 figures, 1 table

Ultrashort-pulse-train pump and dump excitation of a diatomic molecule

OpenAIRE

de Araujo, LEE

2010-01-01

An excitation scheme is proposed for transferring population between ground-vibrational levels of a molecule. The transfer is accomplished by pumping and dumping population with a pair of coherent ultrashort-pulse trains via a stationary state. By mismatching the teeth of the frequency combs associated with the pulse trains to the vibrational levels, high selectivity in the excitation, along with high transfer efficiency, is predicted. The pump-dump scheme does not suffer from spontaneous emi...

Electromagnetic excitation of a generic cavity with a variable e-beam pulse

International Nuclear Information System (INIS)

Fleetwood, R.; Kerris, K.; Merkel, G.; Roberts, H.; Smith, M.

1987-01-01

Relativistic electron-beam nose-erosion techniques have been employed to produce an electron beam with variable pulse shape and bremsstrahlung capability (''dial a pulse''). This capability has been employed to excite a large number of electromagnetic fields inside a canonical cavity. Electron-beam and bremsstrahlung pulse-shape parameters have been varied to produce changes in the electromagnetic cavity response. For example, generic cavity test parameters such as displacement currents or conduction currents can be emphasized or de-emphasized. A theoretical interpretation of these electromagnetic excitations is presented

Modeling pulsed excitation for gas-phase laser diagnostics

International Nuclear Information System (INIS)

Settersten, Thomas B.; Linne, Mark A.

2002-01-01

Excitation dynamics for pulsed optical excitation are described with the density-matrix equations and the rate equations for a two-level system. A critical comparison of the two descriptions is made with complete and consistent formalisms that are amenable to the modeling of applied laser-diagnostic techniques. General solutions, resulting from numerical integration of the differential equations describing the excitation process, are compared for collisional conditions that range from the completely coherent limit to the steady-state limit, for which the two formalisms are identical. This analysis demonstrates the failure of the rate equations to correctly describe the transient details of the excitation process outside the steady-state limit. However, reasonable estimates of the resultant population are obtained for nonsaturating (linear) excitation. This comparison provides the laser diagnostician with the means to evaluate the appropriate model for excitation through a simple picture of the breakdown of the rate-equation validity

Luminescence from ZnSe excited by picosecond mid-infrared FEL pulses

International Nuclear Information System (INIS)

Mitsuyu, T.; Suzuki, T.; Tomimasu, T.

1998-01-01

We have observed blue band-edge emission from a ZnSe crystal under irradiation of mid-infrared picosecond free electron laser (FEL) pulses. The emission characteristics including spectrum, excitation power dependence, excitation wavelength dependence, and decay time have been investigated. The experimental results have indicated that it is difficult to understand the excitation process by multiphoton excitation, thermal excitation, or excitation through mid-gap levels. (Copyright (c) 1998 Elsevier Science B.V., Amsterdam. All rights reserved.)

Pulsed infrared radiation excites cultured neonatal spiral and vestibular ganglion neurons by modulating mitochondrial calcium cycling.

Science.gov (United States)

Lumbreras, Vicente; Bas, Esperanza; Gupta, Chhavi; Rajguru, Suhrud M

2014-09-15

Cochlear implants are currently the most effective solution for profound sensorineural hearing loss, and vestibular prostheses are under development to treat bilateral vestibulopathies. Electrical current spread in these neuroprostheses limits channel independence and, in some cases, may impair their performance. In comparison, optical stimuli that are spatially confined may result in a significant functional improvement. Pulsed infrared radiation (IR) has previously been shown to elicit responses in neurons. This study analyzes the response of neonatal rat spiral and vestibular ganglion neurons in vitro to IR (wavelength = 1,863 nm) using Ca(2+) imaging. Both types of neurons responded consistently with robust intracellular Ca(2+) ([Ca(2+)]i) transients that matched the low-frequency IR pulses applied (4 ms, 0.25-1 pps). Radiant exposures of ∼637 mJ/cm(2) resulted in continual neuronal activation. Temperature or [Ca(2+)] variations in the media did not alter the IR-evoked transients, ruling out extracellular Ca(2+) involvement or primary mediation by thermal effects on the plasma membrane. While blockage of Na(+), K(+), and Ca(2+) plasma membrane channels did not alter the IR-evoked response, blocking of mitochondrial Ca(2+) cycling with CGP-37157 or ruthenium red reversibly inhibited the IR-evoked [Ca(2+)]i transients. Additionally, the magnitude of the IR-evoked transients was dependent on ryanodine and cyclopiazonic acid-dependent Ca(2+) release. These results suggest that IR modulation of intracellular calcium cycling contributes to stimulation of spiral and vestibular ganglion neurons. As a whole, the results suggest selective excitation of neurons in the IR beam path and the potential of IR stimulation in future auditory and vestibular prostheses. Copyright © 2014 the American Physiological Society.

The pulse duration of electrical stimulation influences H-reflexes but not corticospinal excitability for tibialis anterior.

Science.gov (United States)

Hindle, Alyssa R; Lou, Jenny W H; Collins, David F

2014-10-01

The afferent volley generated by neuromuscular electrical stimulation (NMES) influences corticospinal (CS) excitability and frequent NMES sessions can strengthen CS pathways, resulting in long-term improvements in function. This afferent volley can be altered by manipulating NMES parameters. Presently, we manipulated one such parameter, pulse duration, during NMES over the common peroneal nerve and assessed the influence on H-reflexes and CS excitability. We hypothesized that compared with shorter pulse durations, longer pulses would (i) shift the H-reflex recruitment curve to the left, relative to the M-wave curve; and (ii) increase CS excitability more. Using 3 pulse durations (50, 200, 1000 μs), M-wave and H-reflex recruitment curves were collected and, in separate experiments, CS excitability was assessed by comparing motor evoked potentials elicited before and after 30 min of NMES. Despite finding a leftward shift in the H-reflex recruitment curve when using the 1000 μs pulse duration, consistent with a larger afferent volley for a given efferent volley, the increases in CS excitability were not influenced by pulse duration. Hence, although manipulating pulse duration can alter the relative recruitment of afferents and efferents in the common peroneal nerve, under the present experimental conditions it is ineffective for maximizing CS excitability for rehabilitation.

Pulse generator circuit triggerable by nuclear radiation

International Nuclear Information System (INIS)

Fredrickson, P.B.

1980-01-01

A pulse generator circuit triggerable by a pulse of nuclear radiation is described. The pulse generator circuit includes a pair of transistors arranged, together with other electrical components, in the topology of a standard monostable multivibrator circuit. The circuit differs most significantly from a standard monostable multivibrator circuit in that the circuit is adapted to be triggered by a pulse of nuclear radiation rather than electrically and the transistors have substantially different sensitivities to radiation, due to different physical and electrical characteristics and parameters. One of the transistors is employed principally as a radiation detector and is in a normally non-conducting state and the other transistor is normally in a conducting state. When the circuit is exposed to a pulse of nuclear radiation, currents are induced in the collector-base junctions of both transistors but, due to the different radiation sensitivities of the transistors, the current induced in the collector-base junction of the radiation-detecting transistor is substantially greater than that induced in the collector-base junction of the other transistor. The pulse of radiation causes the radiation-detecting transistor to operate in its conducting state, causing the other transistor to operate in its non-conducting state. As the radiation-detecting transistor operates in its conducting state, an output signal is produced at an output terminal connected to the radiation-detecting transistor indicating the presence of a predetermined intensity of nuclear radiation

Characterizing human activity induced impulse and slip-pulse excitations through structural vibration

Science.gov (United States)

Pan, Shijia; Mirshekari, Mostafa; Fagert, Jonathon; Ramirez, Ceferino Gabriel; Chung, Albert Jin; Hu, Chih Chi; Shen, John Paul; Zhang, Pei; Noh, Hae Young

2018-02-01

Many human activities induce excitations on ambient structures with various objects, causing the structures to vibrate. Accurate vibration excitation source detection and characterization enable human activity information inference, hence allowing human activity monitoring for various smart building applications. By utilizing structural vibrations, we can achieve sparse and non-intrusive sensing, unlike pressure- and vision-based methods. Many approaches have been presented on vibration-based source characterization, and they often either focus on one excitation type or have limited performance due to the dispersion and attenuation effects of the structures. In this paper, we present our method to characterize two main types of excitations induced by human activities (impulse and slip-pulse) on multiple structures. By understanding the physical properties of waves and their propagation, the system can achieve accurate excitation tracking on different structures without large-scale labeled training data. Specifically, our algorithm takes properties of surface waves generated by impulse and of body waves generated by slip-pulse into account to handle the dispersion and attenuation effects when different types of excitations happen on various structures. We then evaluate the algorithm through multiple scenarios. Our method achieves up to a six times improvement in impulse localization accuracy and a three times improvement in slip-pulse trajectory length estimation compared to existing methods that do not take wave properties into account.

High-efficiency generation of pulsed Lyman-α radiation by resonant laser wave mixing in low pressure Kr-Ar mixture.

Science.gov (United States)

Saito, Norihito; Oishi, Yu; Miyazaki, Koji; Okamura, Kotaro; Nakamura, Jumpei; Louchev, Oleg A; Iwasaki, Masahiko; Wada, Satoshi

2016-04-04

We report an experimental generation of ns pulsed 121.568 nm Lyman-α radiation by the resonant nonlinear four-wave mixing of 212.556 nm and 845.015 nm radiation pulses providing a high conversion efficiency 1.7x10-3 with the output pulse energy 3.6 μJ achieved using a low pressure Kr-Ar mixture. Theoretical analysis shows that this efficiency is achieved due to the advantage of using (i) the high input laser intensities in combination with (ii) the low gas pressure allowing us to avoid the onset of full-scale discharge in the laser focus. In particular, under our experimental conditions the main mechanism of photoionization caused by the resonant 2-photon 212.556 nm radiation excitation of Kr atoms followed by the 1-photon ionization leads to ≈17% loss of Kr atoms and efficiency loss only by the end of the pulse. The energy of free electrons, generated by 212.556 nm radiation via (2 + 1)-photon ionization and accelerated mainly by 845.015 nm radiation, remains during the pulse below the level sufficient for the onset of full-scale discharge by the electron avalanche. Our analysis also suggests that ≈30-fold increase of 845.015 nm pulse energy can allow one to scale up the L-α radiation pulse energy towards the level of ≈100 μJ.

Repetitively pulsed UV radiation source based on a run-away electron preionised diffuse discharge in nitrogen

Science.gov (United States)

Baksht, E. Kh; Burachenko, A. G.; Lomaev, M. I.; Panchenko, A. N.; Tarasenko, V. F.

2015-04-01

An extended repetitively pulsed source of spontaneous UV radiation is fabricated, which may also be used for producing laser radiation. Voltage pulses with an incident wave amplitude of up to 30 kV, a half-amplitude duration of ~4 ns and a rise time of ~2.5 ns are applied to a gap with a nonuniform electric field. For an excitation region length of 35 cm and a nitrogen pressure of 30 - 760 Torr, a diffusive discharge up to a pulse repetition rate of 2 kHz is produced without using an additional system for gap preionisation. An investigation is made of the plasma of the run-away electron preionised diffuse discharge. Using a CCD camera it is found that the dense diffused plasma fills the gap in a time shorter than 1 ns. X-ray radiation is recorded from behind the foil anode throughout the pressure range under study; a supershort avalanche electron beam is recorded by the collector electrode at pressures below 100 Torr.

Excitation of random intense single-cycle light-pulse chains in optical fiber

International Nuclear Information System (INIS)

Ding, Y C; Zhang, F L; Gao, J B; Chen, Z Y; Lin, C Y; Yu, M Y

2014-01-01

Excitation of intense periodic single-cycle light pulses in a stochastic background arising from continuous wave stimulated Brillouin scattering (SBS) in a long optical fiber with weak optical feedback is found experimentally and modeled theoretically. Such intense light-pulse chains occur randomly and the optical feedback is a requirement for their excitation. The probability of these forms, among the large number of experimental output signals with identifiable waveforms, appearing is only about 3%, with the remainder exhibiting regular SBS characteristics. It is also found that pulses with low period numbers appear more frequently and the probability distribution for their occurrence in terms of the pulse power is roughly L-shaped, like that for rogue waves. The results from a three-wave-coupling model for SBS including feedback phase control agree well qualitatively with the observed phenomena. (paper)

Detection of salmonella on globe fruits using pulse excited magnetoelastic biosensors

Science.gov (United States)

Wikle, Howard C.; Du, Songtao; Prorok, Barton C.; Chin, Bryan A.

2015-05-01

This paper describes the results of a research project to investigate magnetoelastic (ME) biosensors actuated with a pulse excitation to measure the concentration of Salmonella Typhimurium of globe fruits. The ME biosensors are based on an acoustic wave resonator platform that is a freestanding (free-free) thin ribbon of magnetostrictive material with a lengthto- width ratio of 5:1. A biorecognition probe coated on the surface of the resonator platform binds with a targeted pathogen, i.e. E2 phage that binds with S. Typhimurium. The biosensor was actuated to vibrate longitudinally such that the resonant frequency depended primarily on the length of sensor and its overall mass. A pulsed excitation and measurement system was used to actuate micron scale ME biosensors to vibrate. The biosensor responds in a ring-down manner, a damped decay of the resonance amplitude, from which the resonant frequency was measured. An increase in mass due to the binding of the target pathogen resulted in a decrease in the resonant frequency. The pulsed excitation and measurement system that was developed under this effort and the characterization of its performance on the measurement of Salmonella concentrations on globe fruits is described.

Theory of spin and lattice wave dynamics excited by focused laser pulses

Science.gov (United States)

Shen, Ka; Bauer, Gerrit E. W.

2018-06-01

We develop a theory of spin wave dynamics excited by ultrafast focused laser pulses in a magnetic film. We take into account both the volume and surface spin wave modes in the presence of applied, dipolar and magnetic anisotropy fields and include the dependence on laser spot exposure size and magnetic damping. We show that the sound waves generated by local heating by an ultrafast focused laser pulse can excite a wide spectrum of spin waves (on top of a dominant magnon–phonon contribution). Good agreement with recent experiments supports the validity of the model.

Pulse X-radiation in flaw detection

International Nuclear Information System (INIS)

Vavilov, S.P.; Gorbunov, V.I.

1985-01-01

Principles of physical and engineering application of pulse X-radiation (PXR) of micro- and nanosecond duration for nondestructive testing of processes, materials and devices are given. Methods and devices, aimed at generating X-ray pulses, as well as their radiation and flow detection characteristics, and testing methods by means of PXR are considered

ALL-OPTICAL CONTROL OF THZ RADIATION IN PARALLEL PLATE WAVEGUIDES

DEFF Research Database (Denmark)

2010-01-01

The invention relates to control of THz radiation in parallel plate waveguides (PPWG) by forming components in the waveguide by use of optical radiation pulses. Patterns of excited regions induced in the PPWG by an optical excitation pulses changes the electromagnetic properties of the waveguide...... medium in the THz regime, thereby forming transient passive and active components for controlling THz radiation signals. The excitation can be generation of free charge carriers in a semiconductor material in the PPWG, to create metallic regions that form mirrors, lenses or photonic crystal structures......-on-a-chip applications. The optical and THz radiation can be ultrashort pulses with picosecond or femtosecond pulse durations. L...

Luminescent Characteristics of a Pulsed Discharge Plasma in Xe-KBr Mixture

Science.gov (United States)

Heneral, A. A.; Zhmenyak, Y. V.

2018-03-01

A mixture of xenon with a nontoxic halogen carrier Xe-KBr is used to create a plasma radiation source at the 282-nm transition of the XeBr* molecule excited by a high-voltage pulsed-periodic discharge. The luminescence spectra of the plasma of a longitudinal pulsed-periodic discharge in the Xe-KBr mixture at low pressures are studied experimentally. The most intense UV bands of exciplex XeBr* molecules are recorded in the spectral range of 250-350 nm. The spectral, temporal, and energetic characteristics of the radiation source are presented, as well as the dependence of the XeBr* exciplex molecule formation efficiency on the discharge excitation conditions. The optimal conditions for the excitation of UV radiation in the pulsed-periodic discharge plasma are determined.

Improving the efficiency of a fluorescent Xe dielectric barrier light source using short pulse excitation

International Nuclear Information System (INIS)

Beleznai, Sz; Mihajlik, G; Richter, P; Maros, I; Balazs, L

2008-01-01

Operation of a Xe dielectric barrier discharge lamp producing 147-172 nm VUV radiation is investigated both theoretically and experimentally. Xe gas pressure varies between 100 and 300 mbar, and the glass body of the lamp is coated with LAP (green) phosphor to convert radiation into the visible part of the spectrum. Simulation results predict improved discharge efficiencies reaching 67% when excited by a fast rise-time, short pulse (∼200 ns) driving waveform. In this case most power deposited into the plasma efficiently produces Xe 2 * excimers, while other energy dissipation processes (ion heating, e-Xe elastic collision) are kept at a low rate. Simulation and experimental results are compared in terms of discharge efficacy and show good agreement. A lamp efficacy value as high as 80 lm W -1 is demonstrated experimentally

Ultrashort-pulse laser excitation and damage of dielectric materials

DEFF Research Database (Denmark)

Haahr-Lillevang, Lasse; Balling, Peter

2015-01-01

Ultrashort-pulse laser excitation of dielectrics is an intricate problem due to the strong coupling between the rapidly changing material properties and the light. In the present paper, details of a model based on a multiple-rate-equation description of the conduction band are provided. The model...

Pulse excitation experiment of a superconducting generator; chodendo hatsudenki no parusu reiki shiken

Energy Technology Data Exchange (ETDEWEB)

Miyaike, K.; Iimura, T.; Nishimura, M.; Arata, M.; Takabatake, M. [Toshiba Ltd., Tokyo (Japan); Yamada, M.; Kanamori, Y.; Hasegawa, K. [Kansai Electric Power Co., Inc., Osaka (Japan)

1999-11-10

Efficiency improvement, improvement in the stability of electric power system it is miniaturization and weight reduction can be expected in comparison with the traditional-model generator superconducting generator. We produce the small superconducting generator for the experiment experimentally, and performance characteristics verification of the generator is carried out experimentally. This time, pulse excitation test of the superconducting generator was carried out, and the ac loss of the conductor by the pulse excitation investigated the effect on the quenching current. (NEDO)

Pulsed currents carried by whistlers. IV. Electric fields and radiation excited by an electrode

International Nuclear Information System (INIS)

Stenzel, R.L.; Urrutia, J.M.; Rousculp, C.L.

1995-01-01

Electromagnetic properties of current pulses carried by whistler wave packets are obtained from a basic laboratory experiment. While the magnetic field and current density are described in the preceding companion paper (Part III), the present analysis starts with the electric field. The inductive and space charge electric field contributions are separately calculated in Fourier space from the measured magnetic field and Ohm's law along B 0 . Inverse Fourier transformation yields the total electric field in space and time, separated into rotational and divergent contributions. The space-charge density in whistler wave packets is obtained. The cross-field tensor conductivity is determined. The frozen-in condition is nearly satisfied, E+v e xB congruent 0. The dissipation is obtained from Poynting's theorem. The waves are collisionally damped; Landau damping is negligible. A radiation resistance for the electrode is determined. Analogous to Poynting's theorem, the transport of helicity is analyzed. Current helicity is generated by a flow of helicity between pulses traveling in opposite directions which carry opposite signs of helicity. Helicity is dissipated by collisions. These observations complete a detailed description of whistler/current pulses which can occur in various laboratory and space plasmas. copyright 1995 American Institute of Physics

Combining multi-pulse excitation and chirp coding in contrast-enhanced ultrasound imaging

International Nuclear Information System (INIS)

Crocco, M; Sciallero, C; Trucco, A; Pellegretti, P

2009-01-01

The development of techniques to separate the response of the contrast agent from that of the biological tissues is of great importance in ultrasound medical imaging. In the literature, one can find various solutions involving the use of multiple transmitted signals and the weighted sum of related echoes. In this paper, the combination of one of these multi-pulse techniques with a coded excitation is proposed and assessed. Coded excitation has been used mainly to increase the signal-to-noise ratio (SNR) and the penetration depth, provided that a matched filtering is applied in the reception chain. However, it has been shown that a signal with a long duration time also increases the backscattered echoes produced by the microbubbles and, consequently, the contrast-to-tissue ratio. Therefore, the implementation of a multi-pulse technique using a long coded pulse can yield a better contrast-to-tissue ratio and SNR. This paper investigates the combination of the linear chirp pulse with a multi-pulse technique based on the transmission of three pulses. The performance was evaluated using both simulated and real signals, assessing the improvement in the contrast-to-tissue ratio and SNR, the visual quality of the images obtained and the axial accuracy. A comparison with the same multi-pulse technique implemented using a traditional amplitude-modulated pulse revealed that the deployment of a chirp pulse produces several noticeable advantages and only a minor drawback

Repetitively pulsed UV radiation source based on a run-away electron preionised diffuse discharge in nitrogen

Energy Technology Data Exchange (ETDEWEB)

Baksht, E Kh; Burachenko, A G; Lomaev, M I; Panchenko, A N; Tarasenko, V F [Institute of High Current Electronics, Siberian Branch, Russian Academy of Sciences, Tomsk (Russian Federation)

2015-04-30

An extended repetitively pulsed source of spontaneous UV radiation is fabricated, which may also be used for producing laser radiation. Voltage pulses with an incident wave amplitude of up to 30 kV, a half-amplitude duration of ∼4 ns and a rise time of ∼2.5 ns are applied to a gap with a nonuniform electric field. For an excitation region length of 35 cm and a nitrogen pressure of 30 – 760 Torr, a diffusive discharge up to a pulse repetition rate of 2 kHz is produced without using an additional system for gap preionisation. An investigation is made of the plasma of the run-away electron preionised diffuse discharge. Using a CCD camera it is found that the dense diffused plasma fills the gap in a time shorter than 1 ns. X-ray radiation is recorded from behind the foil anode throughout the pressure range under study; a supershort avalanche electron beam is recorded by the collector electrode at pressures below 100 Torr. (laser applications and other topics in quantum electronics)

Lifetime measurement of the cesium 6P3/2 state using ultrafast laser-pulse excitation and ionization

International Nuclear Information System (INIS)

Sell, J. F.; Patterson, B. M.; Ehrenreich, T.; Brooke, G.; Scoville, J.; Knize, R. J.

2011-01-01

We report a precision measurement of the cesium 6P 3/2 excited-state lifetime. Two collimated, counterpropagating thermal Cs beams cross perpendicularly to femtosecond pulsed laser beams. High timing accuracy is achieved from having excitation and ionization laser pulses which originate from the same mode-locked laser. Using pulse selection we vary the separation in time between excitation and ionization laser pulses while counting the ions produced. We obtain a Cs 6P 3/2 lifetime of 30.460(38) ns, which is a factor of two improvement from previous measurements and with an uncertainty of 0.12%, is one of the most accurate lifetime measurements on record.

Suppression of radiation excitation in focusing environment

International Nuclear Information System (INIS)

Huang, Z.; Ruth, R.D.

1996-12-01

Radiation damping and quantum excitation in an electron damping ring and a straight focusing channel are reviewed. They are found to be the two limiting cases in the study of a general bending and focusing combined system. In the intermediate regime where the radiation formation length is comparable to the betatron wavelength, quantum excitation can be exponentially suppressed by focusing field. This new regime may have interesting applications in the generation of ultra-low emittance beams

Efficient method to design RF pulses for parallel excitation MRI using gridding and conjugate gradient.

Science.gov (United States)

Feng, Shuo; Ji, Jim

2014-04-01

Parallel excitation (pTx) techniques with multiple transmit channels have been widely used in high field MRI imaging to shorten the RF pulse duration and/or reduce the specific absorption rate (SAR). However, the efficiency of pulse design still needs substantial improvement for practical real-time applications. In this paper, we present a detailed description of a fast pulse design method with Fourier domain gridding and a conjugate gradient method. Simulation results of the proposed method show that the proposed method can design pTx pulses at an efficiency 10 times higher than that of the conventional conjugate-gradient based method, without reducing the accuracy of the desirable excitation patterns.

Probing spatial properties of electronic excitation in water after interaction with temporally shaped femtosecond laser pulses: Experiments and simulations

Energy Technology Data Exchange (ETDEWEB)

Winkler, Thomas; Sarpe, Cristian; Jelzow, Nikolai [Institute of Physics and CINSaT, University of Kassel, Heinrich-Plett-Str. 40, D-34132 Kassel (Germany); Lillevang, Lasse H. [Department of Physics and Astronomy, Aarhus University, Ny Munkegade 120, DK-8000 Aarhus C (Denmark); Götte, Nadine; Zielinski, Bastian [Institute of Physics and CINSaT, University of Kassel, Heinrich-Plett-Str. 40, D-34132 Kassel (Germany); Balling, Peter [Department of Physics and Astronomy, Aarhus University, Ny Munkegade 120, DK-8000 Aarhus C (Denmark); Senftleben, Arne [Institute of Physics and CINSaT, University of Kassel, Heinrich-Plett-Str. 40, D-34132 Kassel (Germany); Baumert, Thomas, E-mail: baumert@physik.uni-kassel.de [Institute of Physics and CINSaT, University of Kassel, Heinrich-Plett-Str. 40, D-34132 Kassel (Germany)

2016-06-30

Highlights: • Temporally asymmetric shaped femtosecond laser pulses lead to excitation over smaller area and larger depth in water. • Transient optical properties are measured radially resolved by spectral interference in an imaging geometry. • Radially resolved spectral interference shows indications of nonlinear propagation effects at high fluences. - Abstract: In this work, laser excitation of water under ambient conditions is investigated by radially resolved common-path spectral interferometry. Water, as a sample system for dielectric materials, is excited by ultrashort bandwidth-limited and temporally asymmetric shaped femtosecond laser pulses, where the latter start with an intense main pulse followed by a decaying pulse sequence, i.e. a temporal Airy pulse. Spectral interference in an imaging geometry allows measurements of the transient optical properties integrated along the propagation through the sample but radially resolved with respect to the transverse beam profile. Since the optical properties reflect the dynamics of the free-electron plasma, such measurements reveal the spatial characteristics of the laser excitation. We conclude that temporally asymmetric shaped laser pulses are a promising tool for high-precision laser material processing, as they reduce the transverse area of excitation, but increase the excitation inside the material along the beam propagation.

Circuit-field coupled finite element analysis method for an electromagnetic acoustic transducer under pulsed voltage excitation

International Nuclear Information System (INIS)

Hao Kuan-Sheng; Huang Song-Ling; Zhao Wei; Wang Shen

2011-01-01

This paper presents an analytical method for electromagnetic acoustic transducers (EMATs) under voltage excitation and considers the non-uniform distribution of the biased magnetic field. A complete model of EMATs including the non-uniform biased magnetic field, a pulsed eddy current field and the acoustic field is built up. The pulsed voltage excitation is transformed to the frequency domain by fast Fourier transformation (FFT). In terms of the time harmonic field equations of the EMAT system, the impedances of the coils under different frequencies are calculated according to the circuit-field coupling method and Poynting's theorem. Then the currents under different frequencies are calculated according to Ohm's law and the pulsed current excitation is obtained by inverse fast Fourier transformation (IFFT). Lastly, the sequentially coupled finite element method (FEM) is used to calculate the Lorentz force in the EMATs under the current excitation. An actual EMAT with a two-layer two-bundle printed circuit board (PCB) coil, a rectangular permanent magnet and an aluminium specimen is analysed. The coil impedances and the pulsed current are calculated and compared with the experimental results. Their agreement verified the validity of the proposed method. Furthermore, the influences of lift-off distances and the non-uniform static magnetic field on the Lorentz force under pulsed voltage excitation are studied. (interdisciplinary physics and related areas of science and technology)

Implications of electron attachment to highly-excited states in pulsed-power discharges

International Nuclear Information System (INIS)

Pinnaduwage, L.A.; Univ. of Tennessee, Knoxville, TN

1997-01-01

The author points out the possible implications of electron attachment to highly-excited states of molecules in two pulsed power technologies. One involves the pulsed H 2 discharges used for the generation of H ion beams for magnetic fusion energy and particle accelerators. The other is the power modulated plasma discharges used for material processing

Wake-Field Wave Resonant Excitation in Magnetized Plasmas by Electromagnetic Pulse

International Nuclear Information System (INIS)

Milant'ev, V.P.; Turikov, V.A.

2006-01-01

In this paper the space charge wave excitation process at electromagnetic pulse propagation along external magnetic field in vicinity of electron cyclotron resonance. In hydrodynamic approach it is obtained an equation for plasma density under ponderomotive force action. With help of this equation we investigated a wake-field wave amplitude dependence from resonance detuning. The numerical simulation using a PIC method electromagnetic pulse propagation process in the resonant conditions was done

A z-gradient array for simultaneous multi-slice excitation with a single-band RF pulse.

Science.gov (United States)

Ertan, Koray; Taraghinia, Soheil; Sadeghi, Alireza; Atalar, Ergin

2018-07-01

Multi-slice radiofrequency (RF) pulses have higher specific absorption rates, more peak RF power, and longer pulse durations than single-slice RF pulses. Gradient field design techniques using a z-gradient array are investigated for exciting multiple slices with a single-band RF pulse. Two different field design methods are formulated to solve for the required current values of the gradient array elements for the given slice locations. The method requirements are specified, optimization problems are formulated for the minimum current norm and an analytical solution is provided. A 9-channel z-gradient coil array driven by independent, custom-designed gradient amplifiers is used to validate the theory. Performance measures such as normalized slice thickness error, gradient strength per unit norm current, power dissipation, and maximum amplitude of the magnetic field are provided for various slice locations and numbers of slices. Two and 3 slices are excited by a single-band RF pulse in simulations and phantom experiments. The possibility of multi-slice excitation with a single-band RF pulse using a z-gradient array is validated in simulations and phantom experiments. Magn Reson Med 80:400-412, 2018. © 2017 International Society for Magnetic Resonance in Medicine. © 2017 International Society for Magnetic Resonance in Medicine.

Excitation in the radiation chemistry of inorganic gases

International Nuclear Information System (INIS)

Willis, C.; Boyd, A.W.

1976-01-01

Gas phase radiation chemistry yield data and electron impact cross-section data are used to derive excitation mechanisms and to discuss the role of excited states in the radiation chemistry of O 2 , N 2 , N 2 O, CO, CO 2 , H 2 S, H 2 O and NH 3 . For each of these systems available cross-sections for ionization and neutral excitation are listed, together with relevant reaction rate data and a summary of the radiation chemistry studies at both high and low dose rates. In general, fairly complete mechanisms are derived and further tested by energy balance calculations. In order to present as complete a picture as possible, a summary of rates and products of ion-neutralization reactions is given at the end of the paper. (author)

Wave equations for pulse propagation

International Nuclear Information System (INIS)

Shore, B.W.

1987-01-01

Theoretical discussions of the propagation of pulses of laser radiation through atomic or molecular vapor rely on a number of traditional approximations for idealizing the radiation and the molecules, and for quantifying their mutual interaction by various equations of propagation (for the radiation) and excitation (for the molecules). In treating short-pulse phenomena it is essential to consider coherent excitation phenomena of the sort that is manifest in Rabi oscillations of atomic or molecular populations. Such processes are not adequately treated by rate equations for excitation nor by rate equations for radiation. As part of a more comprehensive treatment of the coupled equations that describe propagation of short pulses, this memo presents background discussion of the equations that describe the field. This memo discusses the origin, in Maxwell's equations, of the wave equation used in the description of pulse propagation. It notes the separation into lamellar and solenoidal (or longitudinal and transverse) and positive and negative frequency parts. It mentions the possibility of separating the polarization field into linear and nonlinear parts, in order to define a susceptibility or index of refraction and, from these, a phase and group velocity. The memo discusses various ways of characterizing the polarization characteristics of plane waves, that is, of parameterizing a transverse unit vector, such as the Jones vector, the Stokes vector, and the Poincare sphere. It discusses the connection between macroscopically defined quantities, such as the intensity or, more generally, the Stokes parameters, and microscopic field amplitudes. The material presented here is a portion of a more extensive treatment of propagation to be presented separately. The equations presented here have been described in various books and articles. They are collected here as a summary and review of theory needed when treating pulse propagation

Wave fronts, pulses and wave trains in photoexcited superlattices behaving as excitable or oscillatory media

International Nuclear Information System (INIS)

Arana, J I; Bonilla, L L; Grahn, H T

2011-01-01

Undoped and strongly photoexcited semiconductor superlattices with field-dependent recombination behave as excitable or oscillatory media with spatially discrete nonlinear convection and diffusion. Infinitely long, dc-current-biased superlattices behaving as excitable media exhibit wave fronts with increasing or decreasing profiles, whose velocities can be calculated by means of asymptotic methods. These superlattices can also support pulses of the electric field. Pulses moving downstream with the flux of electrons can be constructed from their component wave fronts, whereas pulses advancing upstream do so slowly and experience saltatory motion: they change slowly in long intervals of time separated by fast transitions during which the pulses jump to the previous superlattice period. Photoexcited superlattices can also behave as oscillatory media and exhibit wave trains. (paper)

The influence of the excitation pulse length on ultrafast magnetization dynamics in nickel

Directory of Open Access Journals (Sweden)

A. Fognini

2015-03-01

Full Text Available The laser-induced demagnetization of a ferromagnet is caused by the temperature of the electron gas as well as the lattice temperature. For long excitation pulses, the two reservoirs are in thermal equilibrium. In contrast to a picosecond laser pulse, a femtosecond pulse causes a non-equilibrium between the electron gas and the lattice. By pump pulse length dependent optical measurements, we find that the magnetodynamics in Ni caused by a picosecond laser pulse can be reconstructed from the response to a femtosecond pulse. The mechanism responsible for demagnetization on the picosecond time scale is therefore contained in the femtosecond demagnetization experiment.

Prospects for coherently driven nuclear radiation by Coulomb excitation

International Nuclear Information System (INIS)

Karamyan, S.A.; Carroll, J.J.

2006-01-01

Possible experiments are discussed in which the Coulomb excitation of nuclear isomers would be followed by sequential energy release. The possibility of the coherent Coulomb excitation of nuclei ensconced in a crystal by channeled relativistic heavy projectiles is considered. The phase shift between neighbor-nuclei excitations can be identical to the photon phase shift for emission in forward direction. Thus, the elementary string of atoms can radiate coherently with emission of characteristic nuclear γ rays and the intensity of the radiation could be increased due to the summation of amplitudes. The Moessbauer conditions should be important for this new type of collective radiation that could be promising in the context of the γ-lasing problem

Excitation of plasma waves by nonlinear currents induced by a high-frequency electromagnetic pulse

Energy Technology Data Exchange (ETDEWEB)

Grishkov, V. E.; Uryupin, S. A., E-mail: uryupin@sci.lebedev.ru [Russian Academy of Sciences, Lebedev Physical Institute (Russian Federation)

2017-03-15

Excitation of plasma waves by nonlinear currents induced by a high-frequency electromagnetic pulse is analyzed within the kinetic approach. It is shown that the most efficient source of plasma waves is the nonlinear current arising due to the gradient of the energy density of the high-frequency field. Generation of plasma waves by the drag current is usually less efficient but not negligibly small at relatively high frequencies of electron–ion collisions. The influence of electron collisions on the excitation of plasma waves by pulses of different duration is described quantitatively.

The interaction with the lower ionosphere of electromagnetic pulses from lightning: Excitation of optical emissions

Science.gov (United States)

Taranenko, Y. N.; Inan, U. S.; Bell, T. F.

1993-01-01

A self consistent and fully kinetic simulation of the interaction of lightning radiated electromagnetic (EM) pulses with the nighttime lower ionosphere indicates that optical emissions observable with conventional instruments would be excited. For example, emissions of the 1st and 2nd positive bands of N2 occur at rates reaching 7 x 10(exp 7) and 10(exp 7) cu cm/s respectively at 92 km altitude for a lightning discharge with an electric field E(sub 100) = 20 V/m (normalized to a 100 km distance). The maximum height integrated intensities of these emissions are 4 x 10(exp 7) and 6 x 10(exp 6) R respectively, lasting for approx. 50 micrometers.

Non-linear excitation of gravitational radiation antennae

International Nuclear Information System (INIS)

Blair, D.G.

1982-01-01

A mechanism of non-linear excitation is proposed to explain observed excess noise in gravitational radiation antennae, driven by low frequency vibration. The mechanism is analogous to the excitation of a violin string by low frequency bowing. Numerical estimates for Weber bars suspended by cables are in good agreement with observations. (Auth.)

Study of ultra-high gradient wakefield excitation by intense ultrashort laser pulses in plasma

International Nuclear Information System (INIS)

Kotaki, Hideyuki

2002-12-01

We investigate a mechanism of nonlinear phenomena in laser-plasma interaction, a laser wakefield excited by intense laser pulses, and the possibility of generating an intense bright electron source by an intense laser pulse. We need to understand and further employ some of these phenomena for our purposes. We measure self-focusing, filamentation, and the anomalous blueshift of the laser pulse. The ionization of gas with the self-focusing causes a broad continuous spectrum with blueshift. The normal blueshift depends on the laser intensity and the plasma density. We, however, have found different phenomenon. The laser spectrum shifts to fixed wavelength independent of the laser power and gas pressure above some critical power. We call the phenomenon 'anomalous blueshift'. The results are explained by the formation of filaments. An intense laser pulse can excite a laser wakefield in plasma. The coherent wakefield excited by 2 TW, 50 fs laser pulses in a gas-jet plasma around 10 18 cm -3 is measured with a time-resolved frequency domain interferometer (FDI). The density distribution of the helium gas is measured with a time-resolved Mach-Zehnder interferometer to search for the optimum laser focus position and timing in the gas-jet. The results show an accelerating wakefield excitation of 20 GeV/m with good coherency, which is useful for ultrahigh gradient particle acceleration in a compact system. This is the first time-resolved measurement of laser wakefield excitation in a gas-jet plasma. The experimental results are compared with a Particle-in-Cell (PIC) simulation. The pump-probe interferometer system of FDI and the anomalous blueshift will be modified to the optical injection system as a relativistic electron beam injector. In 1D PIC simulation we obtain the results of high quality intense electron beam acceleration. These results illuminate the possibility of a high energy and a high quality electron beam acceleration. (author)

SPIDYAN, a MATLAB library for simulating pulse EPR experiments with arbitrary waveform excitation.

Science.gov (United States)

Pribitzer, Stephan; Doll, Andrin; Jeschke, Gunnar

2016-02-01

Frequency-swept chirp pulses, created with arbitrary waveform generators (AWGs), can achieve inversion over a range of several hundreds of MHz. Such passage pulses provide defined flip angles and increase sensitivity. The fact that spectra are not excited at once, but single transitions are passed one after another, can cause new effects in established pulse EPR sequences. We developed a MATLAB library for simulation of pulse EPR, which is especially suited for modeling spin dynamics in ultra-wideband (UWB) EPR experiments, but can also be used for other experiments and NMR. At present the command line controlled SPin DYnamics ANalysis (SPIDYAN) package supports one-spin and two-spin systems with arbitrary spin quantum numbers. By providing the program with appropriate spin operators and Hamiltonian matrices any spin system is accessible, with limits set only by available memory and computation time. Any pulse sequence using rectangular and linearly or variable-rate frequency-swept chirp pulses, including phase cycling can be quickly created. To keep track of spin evolution the user can choose from a vast variety of detection operators, including transition selective operators. If relaxation effects can be neglected, the program solves the Liouville-von Neumann equation and propagates spin density matrices. In the other cases SPIDYAN uses the quantum mechanical master equation and Liouvillians for propagation. In order to consider the resonator response function, which on the scale of UWB excitation limits bandwidth, the program includes a simple RLC circuit model. Another subroutine can compute waveforms that, for a given resonator, maintain a constant critical adiabaticity factor over the excitation band. Computational efficiency is enhanced by precomputing propagator lookup tables for the whole set of AWG output levels. The features of the software library are discussed and demonstrated with spin-echo and population transfer simulations. Copyright © 2016

Observation of a new coherent transient in NMR - nutational two-pulse stimulated echo in the angular distribution of gamma-radiation from oriented nuclei

Energy Technology Data Exchange (ETDEWEB)

Shakhmuratova, L.N.; Hutchison, W.D.; Isbister, D.J.; Chaplin, D.H. [University of New South Wales, Australian Defence Force Academy, School of Physics, University College (Australia)

1997-07-15

A new coherent transient in pulsed NMR, the two-pulse nutational stimulated echo, is reported for the ferromagnetic system {sup 60}CoFe using resonant perturbations on the directional emission of anisotropic gamma-radiation from thermally oriented nuclei. The new spin echo is a result of non-linear nuclear spin dynamics due to large Larmor inhomogeneity active during radiofrequency pulse application. It is made readily observable through the gross detuning between NMR radiofrequency excitation and gamma radiation detection, and inhomogeneity in the Rabi frequency caused by metallic skin-effect. The method of concatenation of perturbation factors in a statistical tensor formalism is quantitatively applied to successfully predict and then fit in detail the experimental time-domain data.

Observation of a new coherent transient in NMR - nutational two-pulse stimulated echo in the angular distribution of gamma-radiation from oriented nuclei

International Nuclear Information System (INIS)

Shakhmuratova, L.N.; Hutchison, W.D.; Isbister, D.J.; Chaplin, D.H.

1997-01-01

A new coherent transient in pulsed NMR, the two-pulse nutational stimulated echo, is reported for the ferromagnetic system 60 CoFe using resonant perturbations on the directional emission of anisotropic gamma-radiation from thermally oriented nuclei. The new spin echo is a result of non-linear nuclear spin dynamics due to large Larmor inhomogeneity active during radiofrequency pulse application. It is made readily observable through the gross detuning between NMR radiofrequency excitation and gamma radiation detection, and inhomogeneity in the Rabi frequency caused by metallic skin-effect. The method of concatenation of perturbation factors in a statistical tensor formalism is quantitatively applied to successfully predict and then fit in detail the experimental time-domain data

Observation of a new coherent transient in NMR -- nutational two-pulse stimulated echo in the angular distribution of γ-radiation from oriented nuclei

Science.gov (United States)

Shakhmuratova, L. N.; Hutchison, W. D.; Isbister, D. J.; Chaplin, D. H.

1997-07-01

A new coherent transient in pulsed NMR, the two-pulse nutational stimulated echo, is reported for the ferromagnetic system 60CoFe using resonant perturbations on the directional emission of anisotropic γ-radiation from thermally oriented nuclei. The new spin echo is a result of non-linear nuclear spin dynamics due to large Larmor inhomogeneity active during radiofrequency pulse application. It is made readily observable through the gross detuning between NMR radiofrequency excitation and gamma radiation detection, and inhomogeneity in the Rabi frequency caused by metallic skin-effect. The method of concatenation of perturbation factors in a statistical tensor formalism is quantitatively applied to successfully predict and then fit in detail the experimental time-domain data.

Multi-pulse orbits and chaotic dynamics in motion of parametrically excited viscoelastic moving belt

International Nuclear Information System (INIS)

Zhang Wei; Yao Minghui

2006-01-01

In this paper, the Shilnikov type multi-pulse orbits and chaotic dynamics of parametrically excited viscoelastic moving belt are studied in detail. Using Kelvin-type viscoelastic constitutive law, the equations of motion for viscoelastic moving belt with the external damping and parametric excitation are given. The four-dimensional averaged equation under the case of primary parametric resonance is obtained by directly using the method of multiple scales and Galerkin's approach to the partial differential governing equation of viscoelastic moving belt. From the averaged equations obtained here, the theory of normal form is used to give the explicit expressions of normal form with a double zero and a pair of pure imaginary eigenvalues. Based on normal form, the energy-phrase method is employed to analyze the global bifurcations and chaotic dynamics in parametrically excited viscoelastic moving belt. The global bifurcation analysis indicates that there exist the heteroclinic bifurcations and the Silnikov type multi-pulse homoclinic orbits in the averaged equation. The results obtained above mean the existence of the chaos for the Smale horseshoe sense in parametrically excited viscoelastic moving belt. The chaotic motions of viscoelastic moving belts are also found by using numerical simulation. A new phenomenon on the multi-pulse jumping orbits is observed from three-dimensional phase space

Spatially periodic structures, under femtosecond pulsed excitation of crystals

International Nuclear Information System (INIS)

Martynovitch, Evgueni F.; Petite, Guillaume; Dresvianski, Vladimir P.; Starchenko, Anton A.

2004-01-01

Measuring the luminescence intensity of specially prepared irradiation defects induced in crystals, we observe that the longitudinal structure of quasi-interferences induced by two orthogonally polarized femtosecond pulses propagating together with different velocities is insensitive to the spatial broadening due to velocity dispersion in the crystals. On the contrary, it does depend on the pulse duration when it is changed by varying the spectral width of the radiation. It thus allows a direct measurement of the coherence time of such pulses. Stability of the axial selectivity is a good sign, taking away a number of serious limitations concerning possible applications

Enhancement of Lamb Wave Imaging Resolution by Step Pulse Excitation and Prewarping

Directory of Open Access Journals (Sweden)

Shangchen Fu

2015-01-01

Full Text Available For the purpose of improving the damage localization accuracy, a prewarping technology is combined with step pulse excitation and this method is used in Lamb wave imaging of plate structures with adjacent damages. Based on the step pulse excitation, various narrowband or burst response can be derived by signal processing technology and this method provides flexibility for further prewarping approach. A narrowband signal warped with a preselected distance is then designed, and the dispersion in the response of this prewarping signal will be greatly reduced. However, in order to calculate the distance for prewarping, the first arrival needs to be estimated from the burst response. From the step-pulse response, narrowband responses at different central frequencies can be obtained, and by averaging peak-value time of their first arrivals, a more accurate estimation can be calculated. By using the prewarping method to the damage scattering signals before imaging, the imaging resolution of the delay-and-sum method can be highly enhanced. The experiment carried out in an aluminum plate with adjacent damages proves the efficiency of this method.

Pulsed magnetic field excitation sensitivity of match-type electric blasting caps

Science.gov (United States)

Parson, Jonathan; Dickens, James; Walter, John; Neuber, Andreas A.

2010-10-01

This paper presents a study on energy deposition and electromagnetic compatibility of match-type electroexplosive devices (EEDs), which recently have found more usage in pulsed power environments with high electromagnetic interference (EMI) background. The sensitivity of these devices makes them dangerous to intended and unintended radiation produced by devices commonly used in pulsed power environments. Match-type EEDs have been found to be susceptible to such low levels of energy (7-8 mJ) that safe operation of these EEDs is vital when in use near devices that produce high levels of pulsed EMI. The scope of this paper is to provide an investigation that incorporates results of similar studies to provide detonation characteristics of these EEDs. The three topics included in this study are sensitivity testing, modeling of the thermodynamic heat propagation, and electromagnetic compatibility from pulsed electromagnetic radiation. The thermodynamic joule heating of the primary explosive has been modeled by a solution to the 1D heat equation. A simple pulsed generator, Marx generator with an inductive load, was used for the electromagnetic compatibility assessment of the coupled field between the pulse generator and shorted EED. The results of the electromagnetic compatibility assessment relate the resistive, inductive, and capacitive components of the pulse generator to the area of the shorted EED.

Pulsed radiation decay logging

International Nuclear Information System (INIS)

Mills, W.R. Jr.

1983-01-01

There are provided new and improved well logging processes and systems wherein the detection of secondary radiation is accomplished during a plurality of time windows in a manner to accurately characterize the decay rate of the secondary radiation. The system comprises a well logging tool having a primary pulsed radiation source which emits repetitive time-spaced bursts of primary radiation and detector means for detecting secondary radiation resulting from the primary radiation and producing output signals in response to the detected radiation. A plurality of measuring channels are provided, each of which produces a count rate function representative of signals received from the detector means during successive time windows occurring between the primary radiation bursts. The logging system further comprises means responsive to the measuring channels for producing a plurality of functions representative of the ratios of the radiation count rates measured during adjacent pairs of the time windows. Comparator means function to compare the ratio functions and select at least one of the ratio functions to generate a signal representative of the decay rate of the secondary radiation

Superluminescence of cadmium sulfide crystals under pulse X-ray radiation

International Nuclear Information System (INIS)

Pavlovskaya, N.G.; Tarasov, M.D.; Balakin, V.A.; Varava, V.P.; Lobov, S.I.; Surskij, O.K.; Tsukerman, V.A.

1977-01-01

Studies were made to elucidate luminescence properties of CdS crystal radiated by short pulses of braking x-ray radiation. Such a radiation causes the appearance of superluminescence. The radiation was carried out at 295 and 170 K, the radiation dose being changed from 3600 to 1600 r/pulse. At the temperature of 295 K light luminescence was registered at the wave length of 528 nm and half-width of 15 nm. While the temperature lowers, the radiation shifts to the range of shorter wave lengths, and a decrease of the spectrum half-width is observed. With the increase of radiation dose the decrease of radiation spectrum half-width is observed. Approximate calculations show that to achieve the spectrum narrowing to 1 nm at room temperature it is necessary to increase radiation dose per pulse 5-6 times

Table-top instrumentation for time-resolved luminescence spectroscopy of solids excited by nanosecond pulse of soft X-ray source and/or UV laser

International Nuclear Information System (INIS)

Bruza, Petr; Fidler, Vlastimil; Nikl, Martin

2011-01-01

The practical applicability of the rare-earth doped scintillators in high-speed detectors is limited by the slow decay components in the temporal response of a scintillator. The study of origin and properties of material defects that induce the slow decay components is of major importance for the development of new scintillation materials. We present a table-top, time-domain UV-VIS luminescence spectrometer, featuring extended time and input sensitivity ranges and two excitation sources. The combination of both soft X-ray/XUV and UV excitation source allows the comparative measurements of luminescence spectra and decay kinetics of scintillators to be performed under the same experimental conditions. The luminescence of emission centers of a doped scintillator can be induced by conventional N 2 laser pulse, while the complete scintillation process can be initiated by a soft X-ray/XUV pulse excitation from the laser-produced plasma in gas puff target of 4 ns duration. In order to demonstrate the spectrometer, the UV-VIS luminescence spectra and decay kinetics of cerium doped Lu 3 Al 5 O 12 single crystal (LuAG:Ce) scintillator excited by XUV and UV radiation were acquired. Luminescence of the doped Ce 3+ ions was studied under 2.88 nm (430 eV) XUV excitation from the laser-produced nitrogen plasma, and compared with the luminescence under 337 nm (3.68 eV) UV excitation from nitrogen laser. In the former case the excitation energy is deposited in the LuAG host, while in the latter the 4f-5d 2 transition of Ce 3+ is directly excited. Furthermore, YAG:Ce and LuAG:Ce single crystals luminescence decay profiles are compared and discussed.

Electrical pulse burnout of transistors in intense ionizing radiation

International Nuclear Information System (INIS)

Hartman, E.F.; Evans, D.C.

1975-01-01

Tests examining possible synergistic effects of electrical pulses and ionizing radiation on transistors were performed and energy/power thresholds for transistor burnout determined. The effect of ionizing radiation on burnout thresholds was found to be minimal, indicating that electrical pulse testing in the absence of radiation produces burnout-threshold results which are applicable to IEMP studies. The conditions of ionized transistor junctions and radiation induced current surges at semiconductor device terminals are inherent in IEMP studies of electrical circuits

Macrophage and tumor cell responses to repetitive pulsed X-ray radiation

Science.gov (United States)

Buldakov, M. A.; Tretyakova, M. S.; Ryabov, V. B.; Klimov, I. A.; Kutenkov, O. P.; Kzhyshkowska, J.; Bol'shakov, M. A.; Rostov, V. V.; Cherdyntseva, N. V.

2017-05-01

To study a response of tumor cells and macrophages to the repetitive pulsed low-dose X-ray radiation. Methods. Tumor growth and lung metastasis of mice with an injected Lewis lung carcinoma were analysed, using C57Bl6. Monocytes were isolated from a human blood, using CD14+ magnetic beads. IL6, IL1-betta, and TNF-alpha were determined by ELISA. For macrophage phenotyping, a confocal microscopy was applied. “Sinus-150” was used for the generation of pulsed X-ray radiation (the absorbed dose was below 0.1 Gy, the pulse repetition frequency was 10 pulse/sec). The irradiation of mice by 0.1 Gy pulsed X-rays significantly inhibited the growth of primary tumor and reduced the number of metastatic colonies in the lung. Furthermore, the changes in macrophage phenotype and cytokine secretion were observed after repetitive pulsed X-ray radiation. Conclusion. Macrophages and tumor cells had a different response to a low-dose pulsed X-ray radiation. An activation of the immune system through changes of a macrophage phenotype can result in a significant antitumor effect of the low-dose repetitive pulsed X-ray radiation.

Application of adjustable pulse lasers to studying rapid reaction kinetics of excited lanthanide complexing

Energy Technology Data Exchange (ETDEWEB)

Gruzdev, V.P. (Gosudarstvennyj Opticheskij Inst., Leningrad (USSR))

1983-12-01

Using some europium (3) ion complexes new possibilities to be opened by application of adjustable pulse lasers for studying rapid reactions of electron-excited metal ion complexing are demonstrated. The 6Zh rhodamine pulse laser is used as a source of nonequilibrium photoexcitation of an array of Eu/sup 3 +/ complexes in the luminescent kinetic spectroscopy method. The following results are obtained: for the first time the rate of reaction of acetate ion substitution for water molecules of an excited (/sup 5/D/sub 0/) ion of Eu/sup 3 +/ was measured to be (0.7+-0.2)x10/sup 7/ s/sup -1/; using direct experiments the lower limit for the rate of transition of one isomeric form of the excited Eu x EDTA complex into another one in an aqueous solution is determined to be 5x10/sup 5/ s/sup -1/ at 295 K; the kinetics of the excitation energy migration beteen aqueous solvates of Eu/sup 3 +/ and EuxEDTA complexes is investigated.

Cherenkov excited phosphorescence-based pO2 estimation during multi-beam radiation therapy: phantom and simulation studies.

Science.gov (United States)

Holt, Robert W; Zhang, Rongxiao; Esipova, Tatiana V; Vinogradov, Sergei A; Glaser, Adam K; Gladstone, David J; Pogue, Brian W

2014-09-21

Megavoltage radiation beams used in External Beam Radiotherapy (EBRT) generate Cherenkov light emission in tissues and equivalent phantoms. This optical emission was utilized to excite an oxygen-sensitive phosphorescent probe, PtG4, which has been developed specifically for NIR lifetime-based sensing of the partial pressure of oxygen (pO2). Phosphorescence emission, at different time points with respect to the excitation pulse, was acquired by an intensifier-gated CCD camera synchronized with radiation pulses delivered by a medical linear accelerator. The pO2 distribution was tomographically recovered in a tissue-equivalent phantom during EBRT with multiple beams targeted from different angles at a tumor-like anomaly. The reconstructions were tested in two different phantoms that have fully oxygenated background, to compare a fully oxygenated and a fully deoxygenated inclusion. To simulate a realistic situation of EBRT, where the size and location of the tumor is well known, spatial information of a prescribed region was utilized in the recovery estimation. The phantom results show that region-averaged pO2 values were recovered successfully, differentiating aerated and deoxygenated inclusions. Finally, a simulation study was performed showing that pO2 in human brain tumors can be measured to within 15 mmHg for edge depths less than 10-20 mm using the Cherenkov Excited Phosphorescence Oxygen imaging (CEPhOx) method and PtG4 as a probe. This technique could allow non-invasive monitoring of pO2 in tumors during the normal process of EBRT, where beams are generally delivered from multiple angles or arcs during each treatment fraction.

Selective reflection of resonance radiation from excited media

International Nuclear Information System (INIS)

Veklenko, B.A.; Gusarov, R.B.; Sherkunov, Yu.B.

1998-01-01

According to quantum electrodynamics, the cross section for resonant scattering of radiation on an aggregate of excited atoms can be written as a sum of positive definite terms. This type of structure is not consistent with the Fresnel formulas for the reflection coefficient of radiation from thermally excited media. The difference shows up on a macroscopic level and indicates that semiclassical radiation theory cannot be used. A study of the correlation between elastic scattering and stimulated emission processes clarifies the reason for the discrepancies. The resulting singularities require summing of Feynman diagrams which appear beginning in the sixth order of perturbation theory. A lower bound estimate for the reflection coefficient from a plane layer is given, including processes which violate the statistics of radiation. The contribution of stimulated emission processes caused by the initially scattered photon are examined specifically. An experiment is proposed which would settle the choice of theories

Subfemtosecond pulse generation by cascade-stimulated Raman scattering with modulated Raman excitation

International Nuclear Information System (INIS)

Wu Kun; Wu Jian; Zeng Heping

2003-01-01

Subfemtosecond (sub-fs) pulses can be generated by cascade-stimulated Raman scattering in a Raman medium with modulated Raman excitations, driven by two sufficiently intense laser beams, one of which is amplitude modulated. The nonadiabatic Raman interaction establishes a strong modulated Raman coherence, which supports compression of the generated broadband Raman sidebands to a train of sub-fs pulses regardless of whether the carrier frequencies of the driving lasers are tuned above, below or on two-photon Raman resonance. (letter to the editor)

Femto-second pulses of synchrotron radiation

International Nuclear Information System (INIS)

Zholents, A.A.; Zolotorev, M.S.

1995-07-01

A method capable of producing femto-second pulses of synchrotron radiation is proposed. It is based on the interaction of femto-second light pulses with electrons in a storage ring. The application of the method to the generation of ultra-short x-ray pulses at the Advance Light Source of Lawrence Berkeley National Laboratory has been considered. The same method can also be used for extraction of electrons from a storage ring in ultra-short series of microbunches spaced by the periodicity of light wavelength

Nuclear Excitation by a Zeptosecond Multi-MeV Laser Pulse

International Nuclear Information System (INIS)

Weidenmueller, Hans A.

2011-01-01

A zeptosecond multi-MeV laser pulse may either excite a ''plasma'' of strongly interacting nucleons or a collective mode. We derive the conditions on laser energy and photon number such that either of these scenarios is realized. We use the nuclear giant dipole resonance as a representative example, and a random-matrix description of the fine-structure states and perturbation theory as tools.

A fast pulse design for parallel excitation with gridding conjugate gradient.

Science.gov (United States)

Feng, Shuo; Ji, Jim

2013-01-01

Parallel excitation (pTx) is recognized as a crucial technique in high field MRI to address the transmit field inhomogeneity problem. However, it can be time consuming to design pTx pulses which is not desirable. In this work, we propose a pulse design with gridding conjugate gradient (CG) based on the small-tip-angle approximation. The two major time consuming matrix-vector multiplications are substituted by two operators which involves with FFT and gridding only. Simulation results have shown that the proposed method is 3 times faster than conventional method and the memory cost is reduced by 1000 times.

Laser excitation of SF6: spectroscopy and coherent pulse propagation effects

International Nuclear Information System (INIS)

Cantrell, C.D.; Makarov, A.A.; Louisell, W.H.

1978-01-01

Recent theoretical studies of coherent propagation effects in SF 6 and other polyatomic molecules are summarized beginning with an account of relevant aspects of the high-resolution spectroscopy of the ν 3 band of SF 6 . A laser pulse propagating in a molecular gas can acquire new frequencies which were not initially present in the pulse, and, in fact, a wave is coherently generated at the frequency of every molecular transition accessible from the initial molecular energy levels. The possible consequences of coherent generation of sidebands for the multiple-photon excitation of SF 6 and other polyatomic molecules are discussed

Effective excitation of DBD lamp with a long feedline

International Nuclear Information System (INIS)

Schitz, D V; Nechoroshev, V O

2016-01-01

The proposed solution makes possible the transfer of high-voltage excitation pulses through the long coaxial cable with the minimum losses and the excilamp efficiency. Use of resonant topology of the pulse converter provides ZCS at switching-ON and ZVC at switching- OFF of the transistors. The values of efficiency of radiation of ∼ 9% at the feedline of 2.5 m in length obtained during the experiments are about twice as much as the efficiency at the XeCl- excilamp excitation by the quasi-square pulses power supply due to the decrease of losses at switching and the increase of electric efficiency of a resonant power supply with the long coaxial feedline. (paper)

Biomolecular ligands screening using radiation damping difference WaterLOGSY spectroscopy

International Nuclear Information System (INIS)

Sun Peng; Jiang Xianwang; Jiang Bin; Zhang Xu; Liu Maili

2013-01-01

Water-ligand observed via gradient spectroscopy (WaterLOGSY) is a widely used nuclear magnetic resonance method for ligand screening. The crucial procedure for the effectiveness of WaterLOGSY is selective excitation of the water resonance. The selective excitation is conventionally achieved by using long selective pulse, which causes partial saturation of the water magnetization leading to reduction of sensitivity, in addition to time consuming and error prone. Therefore, many improvements have been made to enhance the sensitivity and robustness of the method. Here we propose an alternative selective excitation scheme for WaterLOGSY by utilizing radiation damping effect. The pulse scheme starts simply with a hard inversion pulse, instead of selective pulse or pulse train, followed by a pulse field gradient to control the radiation damping effect. The rest parts of the pulse scheme are similar to conventional WaterLOGSY. When the gradient pulse is applied immediately after the inversion pulse, the radiation damping effect is suppressed, and all of the magnetization is inversed. When the gradient pulse and the inversion pulse are about 10–20 ms apart, the radiation damping effect remains active and drives the water magnetization toward +z-axis, resulting in selective non-inversion of the water magnetization. By taking the differences of the spectra obtained under these two conditions, one should get the result of WaterLOGSY. The method is demonstrated to be simple, robust and sensitive for ligand screening

Asymmetric noise sensitivity of pulse trains in an excitable microlaser with delayed optical feedback

Science.gov (United States)

Terrien, Soizic; Krauskopf, Bernd; Broderick, Neil G. R.; Andréoli, Louis; Selmi, Foued; Braive, Rémy; Beaudoin, Grégoire; Sagnes, Isabelle; Barbay, Sylvain

2017-10-01

A semiconductor micropillar laser with delayed optical feedback is considered. In the excitable regime, we show that a single optical perturbation can trigger a train of pulses that is sustained for a finite duration. The distribution of the pulse train duration exhibits an exponential behavior characteristic of a noise-induced process driven by uncorrelated white noise present in the system. The comparison of experimental observations with theoretical and numerical analysis of a minimal model yields excellent agreement. Importantly, the random switch-off process takes place between two attractors of different nature: an equilibrium and a periodic orbit. Our analysis shows that there is a small time window during which the pulsations are very sensitive to noise, and this explains the observed strong bias toward switch-off. These results raise the possibility of all optical control of the pulse train duration that may have an impact for practical applications in photonics and may also apply to the dynamics of other noise-driven excitable systems with delayed feedback.

Radiation and propagation of short acoustical pulses from underground explosions

International Nuclear Information System (INIS)

Banister, J.R.

1982-06-01

Radiation and propagation of short acoustical pulses from underground nuclear explosions were analyzed. The cone of more intense radiation is defined by the ratio of sound speeds in the ground and air. The pressure history of the radiated pulse is a function of the vertical ground-motion history, the range, the burial depth, and the velocity of longitudinal seismic waves. The analysis of short-pulse propagation employed an N-wave model with and without enegy conservation. Short pulses with initial wave lengths less than 100 m are severely attenuated by the energy loss in shocks and viscous losses in the wave interior. The methods developed in this study should be useful for system analysis

A Bit Stream Scalable Speech/Audio Coder Combining Enhanced Regular Pulse Excitation and Parametric Coding

Directory of Open Access Journals (Sweden)

Albertus C. den Brinker

2007-01-01

Full Text Available This paper introduces a new audio and speech broadband coding technique based on the combination of a pulse excitation coder and a standardized parametric coder, namely, MPEG-4 high-quality parametric coder. After presenting a series of enhancements to regular pulse excitation (RPE to make it suitable for the modeling of broadband signals, it is shown how pulse and parametric codings complement each other and how they can be merged to yield a layered bit stream scalable coder able to operate at different points in the quality bit rate plane. The performance of the proposed coder is evaluated in a listening test. The major result is that the extra functionality of the bit stream scalability does not come at the price of a reduced performance since the coder is competitive with standardized coders (MP3, AAC, SSC.

A Bit Stream Scalable Speech/Audio Coder Combining Enhanced Regular Pulse Excitation and Parametric Coding

Science.gov (United States)

Riera-Palou, Felip; den Brinker, Albertus C.

2007-12-01

This paper introduces a new audio and speech broadband coding technique based on the combination of a pulse excitation coder and a standardized parametric coder, namely, MPEG-4 high-quality parametric coder. After presenting a series of enhancements to regular pulse excitation (RPE) to make it suitable for the modeling of broadband signals, it is shown how pulse and parametric codings complement each other and how they can be merged to yield a layered bit stream scalable coder able to operate at different points in the quality bit rate plane. The performance of the proposed coder is evaluated in a listening test. The major result is that the extra functionality of the bit stream scalability does not come at the price of a reduced performance since the coder is competitive with standardized coders (MP3, AAC, SSC).

TH-C-17A-05: Cherenkov Excited Phosphorescence Oxygen (CEPhOx) Imaging During Multi-Beam Radiation Therapy

Energy Technology Data Exchange (ETDEWEB)

Zhang, R; Pogue, B [Dartmouth College, Hanover, NH (United States); Holt, R [Dartmouth College, Hanover, NH - New Hampshire (United States); Esipova, T; Vinogradov, S [University of Pennsylvania, Philadelphia, PA (United States); Gladstone, D [Dartmouth-Hitchcock Medical Center, Hanover, City of Lebanon (Lebanon)

2014-06-15

Purpose: Cherenkov radiation is created during external beam radiation therapy that can excite phosphorescence in tissue from oxygen-sensitive, bio-compatible probes. Utilizing the known spatial information of the treatment plan with directed multiple beam angles, Cherenkov Excited Phosphorescence Oxygen (CEPhOx) imaging was realized from the reconstructions of Cherenkov excited phosphorescence lifetime. Methods: Platinum(II)-G4 (PtG4) was used as the oxygen-sensitive phosphorescent probe and added to a oxygenated cylindrical liquid phantom with a oxygenated/deoxygenated cylindrical anomaly. Cherenkov excited phosphorescence was imaged using a time-gated ICCD camera temporallysynchronized to the LINAC pulse output. Lifetime reconstruction was carried out in NIRFAST software. Multiple angles of the incident radiation beam was combined with the location of the prescribed treatment volume (PTV) to improve the tomographic recovery as a function of location. The tissue partial pressure of oxygen (pO2) in the background and PTV was calculated based on the recovered lifetime distribution and Stern-Volmer equation. Additionally a simulation study was performed to examine the accuracy of this technique in the setting of a human brain tumor. Results: Region-based pO2 values in the oxygenated background and oxygenated/deoxygenated PTV were correctly recovered, with the deoxygenated anomaly (15.4 mmHg) easily distinguished from the oxygenated background (143 mmHg). The data acquisition time could be achieved within the normal irradiation time for a human fractionated plan. The simulations indicated that CEPhOx would be a sufficient to sample tumor pO2 sensing from tumors which are larger than 2cm in diameter or within 23mm depth from the surface. Conclusion: CEPhOx could be a novel imaging tool for pO2 assessment during external radiation beam therapy. It is minimally invasive and should work within the established treatment plan of radiation therapy with multiple beams in

The effect of excitation and preparation pulses on nonslice selective 2D UTE bicomponent analysis of bound and free water in cortical bone at 3T

Energy Technology Data Exchange (ETDEWEB)

Li, Shihong [Department of Radiology, University of California, San Diego, California 92103-8226 (United States); Department of Radiology, Hua Dong Hospital, Fudan University, Shanghai 200040 (China); Yancheng Medical College, Jiangsu (China); The First People' s Hospital of Yancheng City, Jiangsu 224005 (China); Chang, Eric Y.; Chung, Christine B. [VA San Diego Healthcare System, San Diego, California 92161 and Department of Radiology, University of California, San Diego, California 92103-8226 (United States); Bae, Won C.; Du, Jiang, E-mail: jiangdu@ucsd.edu [Department of Radiology, University of California, San Diego, California 92103-8226 (United States); Hua, Yanqing [Department of Radiology, Hua Dong Hospital, Fudan University, Shanghai 200040 (China); Zhou, Yi [The First People' s Hospital of Yancheng City, Jiangsu 224005 (China)

2014-02-15

Purpose: The purpose of this study was to investigate the effect of excitation, fat saturation, long T2 saturation, and adiabatic inversion pulses on ultrashort echo time (UTE) imaging with bicomponent analysis of bound and free water in cortical bone for potential applications in osteoporosis. Methods: Six bovine cortical bones and six human tibial midshaft samples were harvested for this study. Each bone sample was imaged with eight sequences using 2D UTE imaging at 3T with half and hard excitation pulses, without and with fat saturation, long T2 saturation, and adiabatic inversion recovery (IR) preparation pulses. Single- and bicomponent signal models were utilized to calculate the T2{sup *}s and/or relative fractions of short and long T2{sup *}s. Results: For all bone samples UTE T2{sup *} signal decay showed bicomponent behavior. A higher short T2{sup *} fraction was observed on UTE images with hard pulse excitation compared with half pulse excitation (75.6% vs 68.8% in bovine bone, 79.9% vs 73.2% in human bone). Fat saturation pulses slightly reduced the short T2{sup *} fraction relative to regular UTE sequences (5.0% and 2.0% reduction, respectively, with half and hard excitation pulses for bovine bone, 6.3% and 8.2% reduction, respectively, with half and hard excitation pulses for human bone). Long T2 saturation pulses significantly reduced the long T2{sup *} fraction relative to regular UTE sequence (18.9% and 17.2% reduction, respectively, with half and hard excitation pulses for bovine bone, 26.4% and 27.7% reduction, respectively, with half and hard excitation pulses for human bone). With IR-UTE preparation the long T2{sup *} components were significantly reduced relative to regular UTE sequence (75.3% and 66.4% reduction, respectively, with half and hard excitation pulses for bovine bone, 87.7% and 90.3% reduction, respectively, with half and hard excitation pulses for human bone). Conclusions: Bound and free water T2{sup *}s and relative fractions can

The effect of excitation and preparation pulses on nonslice selective 2D UTE bicomponent analysis of bound and free water in cortical bone at 3T

International Nuclear Information System (INIS)

Li, Shihong; Chang, Eric Y.; Chung, Christine B.; Bae, Won C.; Du, Jiang; Hua, Yanqing; Zhou, Yi

2014-01-01

Purpose: The purpose of this study was to investigate the effect of excitation, fat saturation, long T2 saturation, and adiabatic inversion pulses on ultrashort echo time (UTE) imaging with bicomponent analysis of bound and free water in cortical bone for potential applications in osteoporosis. Methods: Six bovine cortical bones and six human tibial midshaft samples were harvested for this study. Each bone sample was imaged with eight sequences using 2D UTE imaging at 3T with half and hard excitation pulses, without and with fat saturation, long T2 saturation, and adiabatic inversion recovery (IR) preparation pulses. Single- and bicomponent signal models were utilized to calculate the T2 * s and/or relative fractions of short and long T2 * s. Results: For all bone samples UTE T2 * signal decay showed bicomponent behavior. A higher short T2 * fraction was observed on UTE images with hard pulse excitation compared with half pulse excitation (75.6% vs 68.8% in bovine bone, 79.9% vs 73.2% in human bone). Fat saturation pulses slightly reduced the short T2 * fraction relative to regular UTE sequences (5.0% and 2.0% reduction, respectively, with half and hard excitation pulses for bovine bone, 6.3% and 8.2% reduction, respectively, with half and hard excitation pulses for human bone). Long T2 saturation pulses significantly reduced the long T2 * fraction relative to regular UTE sequence (18.9% and 17.2% reduction, respectively, with half and hard excitation pulses for bovine bone, 26.4% and 27.7% reduction, respectively, with half and hard excitation pulses for human bone). With IR-UTE preparation the long T2 * components were significantly reduced relative to regular UTE sequence (75.3% and 66.4% reduction, respectively, with half and hard excitation pulses for bovine bone, 87.7% and 90.3% reduction, respectively, with half and hard excitation pulses for human bone). Conclusions: Bound and free water T2 * s and relative fractions can be assessed using UTE bicomponent

Vibration control in smart coupled beams subjected to pulse excitations

Science.gov (United States)

Pisarski, Dominik; Bajer, Czesław I.; Dyniewicz, Bartłomiej; Bajkowski, Jacek M.

2016-10-01

In this paper, a control method to stabilize the vibration of adjacent structures is presented. The control is realized by changes of the stiffness parameters of the structure's couplers. A pulse excitation applied to the coupled adjacent beams is imposed as the kinematic excitation. For such a representation, the designed control law provides the best rate of energy dissipation. By means of a stability analysis, the performance in different structural settings is studied. The efficiency of the proposed strategy is examined via numerical simulations. In terms of the assumed energy metric, the controlled structure outperforms its passively damped equivalent by over 50 percent. The functionality of the proposed control strategy should attract the attention of practising engineers who seek solutions to upgrade existing damping systems.

Electromagnetic radiation of ultrarelativistic particles at scattering in excited medium

International Nuclear Information System (INIS)

Malyshevskij, V.S.

1990-01-01

The interaction between relativistic particles and a gaseous or condensed medium with a high density of nondegenerate excited quantum states involves the coherent conversion of atomic or molecular excitations into electromagnetic radiation

Relaxation and excitation electronic processes in dielectrics irradiated by ultrafast IR and VUV pulses

International Nuclear Information System (INIS)

Gaudin, J.

2005-11-01

We studied excitation and relaxation of electrons involved during interaction of visible and VUV femtosecond pulses with dielectrics. The generated population of hot electrons, having energy of few eV to few tens of eV above the bottom of the conduction band, is responsible of phenomena ranging to defect creation to optical breakdown. Owing to two techniques: photoemission and transient photoconductivity we improve the understanding of the The first photoemission experiments deal with dielectrics irradiated by 30 fs IR pulses. The photoemission spectra measured show a large population of electrons which energy rise up to 40 eV. We interpret this result in terms of a new absorption process: direct multi-photons inter-branch transitions. The 2. type of photoemission experiments are time resolved 'pump/probe' investigation. We study the relaxation of electrons excited by a VUV pulses. We used the high order harmonics (HOH) as light sources. We found surprisingly long decay time in the range of ps timescale. Last type of experiments is photoconductivity studies of diamond samples. Using HOH as light source we measure the displacement current induced by excited electrons in the conduction band. Those electrons relax mainly by impact ionisation creating secondary electrons. Hence by probing the number of electrons we were able to measure the efficiency of these relaxation processes. We observe a diminution of this efficiency when the energy of exciting photons is above 20 eV. Owing to Monte-Carlo simulation we interpret this result in terms of band structure effect. (author)

High excitation of the species in nitrogen–aluminum plasma generated by electron cyclotron resonance microwave discharge of N2 gas and pulsed laser ablation of Al target

International Nuclear Information System (INIS)

Liang, Peipei; Li, Yanli; Cai, Hua; You, Qinghu; Yang, Xu; Huang, Feiling; Sun, Jian; Xu, Ning; Wu, Jiada

2014-01-01

A reactive nitrogen–aluminum plasma generated by electron cyclotron resonance (ECR) microwave discharge of N 2 gas and pulsed laser ablation of an Al target is characterized spectroscopically by time-integrated and time-resolved optical emission spectroscopy (OES). The vibrational and rotational temperatures of N 2 species are determined by spectral simulation. The generated plasma strongly emits radiation from a variety of excited species including ambient nitrogen and ablated aluminum and exhibits unique features in optical emission and temperature evolution compared with the plasmas generated by a pure ECR discharge or by the expansion of the ablation plume. The working N 2 gas is first excited by ECR discharge and the excitation of nitrogen is further enhanced due to the fast expansion of the aluminum plume induced by target ablation, while the excitation of the ablated aluminum is prolonged during the plume expansion in the ECR nitrogen plasma, resulting in the formation of strongly reactive nitrogen–aluminum plasma which contains highly excited species with high vibrational and rotational temperatures. The enhanced intensities and the prolonged duration of the optical emissions of the combined plasma would provide an improved analytical capability for spectrochemical analysis. - Highlights: • ECR discharge and pulsed laser ablation generate highly excited ECR–PLA plasma. • The expansion of PLA plasma results in excitation enhancement of ECR plasma species. • The ECR plasma leads to excitation prolongation of PLA plasma species. • The ECR–PLA plasma emits strong emissions from a variety of excited species. • The ECR–PLA plasma maintains high vibrational–rotational temperatures for a long time

Remotely Exploring Deeper-Into-Matter by Non-Contact Detection of Audible Transients Excited by Laser Radiation

Directory of Open Access Journals (Sweden)

Javier Moros

2017-12-01

Full Text Available An acoustic spectroscopic approach to detect contents within different packaging, with substantially wider applicability than other currently available subsurface spectroscopies, is presented. A frequency-doubled Nd:YAG (neodymium-doped yttrium aluminum garnet pulsed laser (13 ns pulse length operated at 1 Hz was used to generate the sound field of a two-component system at a distance of 50 cm. The acoustic emission was captured using a unidirectional microphone and analyzed in the frequency domain. The focused laser pulse hitting the system, with intensity above that necessary to ablate the irradiated surface, transferred an impulsive force which led the structure to vibrate. Acoustic airborne transients were directly radiated by the vibrating elastic structure of the outer component that excited the surrounding air in contact with. However, under boundary conditions, sound field is modulated by the inner component that modified the dynamical integrity of the system. Thus, the resulting frequency spectra are useful indicators of the concealed content that influences the contributions originating from the wall of the container. High-quality acoustic spectra could be recorded from a gas (air, liquid (water, and solid (sand placed inside opaque chemical-resistant polypropylene and stainless steel sample containers. Discussion about effects of laser excitation energy and sampling position on the acoustic emission events is reported. Acoustic spectroscopy may complement the other subsurface alternative spectroscopies, severely limited by their inherent optical requirements for numerous detection scenarios.

Discrete excitation of mode pulses using a diode-pumped solid-state digital laser

CSIR Research Space (South Africa)

Ngcobo, Sandile

2016-02-01

Full Text Available In this paper, we experimentally demonstrate novel method of generating discrete excitation of on-demand Lagaurre-Gaussian (LG) mode pulses, in a diode pumped solid-state digital laser. The digital laser comprises of an intra-cavity spatial light...

Slice-selective RF pulses for in vivo B1+ inhomogeneity mitigation at 7 tesla using parallel RF excitation with a 16-element coil.

Science.gov (United States)

Setsompop, Kawin; Alagappan, Vijayanand; Gagoski, Borjan; Witzel, Thomas; Polimeni, Jonathan; Potthast, Andreas; Hebrank, Franz; Fontius, Ulrich; Schmitt, Franz; Wald, Lawrence L; Adalsteinsson, Elfar

2008-12-01

Slice-selective RF waveforms that mitigate severe B1+ inhomogeneity at 7 Tesla using parallel excitation were designed and validated in a water phantom and human studies on six subjects using a 16-element degenerate stripline array coil driven with a butler matrix to utilize the eight most favorable birdcage modes. The parallel RF waveform design applied magnitude least-squares (MLS) criteria with an optimized k-space excitation trajectory to significantly improve profile uniformity compared to conventional least-squares (LS) designs. Parallel excitation RF pulses designed to excite a uniform in-plane flip angle (FA) with slice selection in the z-direction were demonstrated and compared with conventional sinc-pulse excitation and RF shimming. In all cases, the parallel RF excitation significantly mitigated the effects of inhomogeneous B1+ on the excitation FA. The optimized parallel RF pulses for human B1+ mitigation were only 67% longer than a conventional sinc-based excitation, but significantly outperformed RF shimming. For example the standard deviations (SDs) of the in-plane FA (averaged over six human studies) were 16.7% for conventional sinc excitation, 13.3% for RF shimming, and 7.6% for parallel excitation. This work demonstrates that excitations with parallel RF systems can provide slice selection with spatially uniform FAs at high field strengths with only a small pulse-duration penalty. (c) 2008 Wiley-Liss, Inc.

Enhanced Electron Attachment to Highly-Excited Molecules and Its Applications in Pulsed Plasmas

International Nuclear Information System (INIS)

Ding, W.X.; Ma, C.Y.; McCorkle, D.L.; Pinnaduwage, L.A.

1999-01-01

Studies conducted over the past several years have shown that electron attachment to highly-excited states of molecules have extremely large cross sections. We will discuss the implications of this for pulsed discharges used for H - generation, material processing, and plasma remediation

Selective photoionization of isotopic atoms with pulsed lasers

International Nuclear Information System (INIS)

Dai Changjian

1994-01-01

The dynamics of isotopically selective interactions between the radiation of three pulsed lasers and atoms with a four-levels scheme has been studied. Starting from the time-dependent Schroedinger equation with the rotating-wave approximation, authors applied Sylvester theorem to the dynamic equations associated with near-and off-resonant excitations, respectively. Authors obtained the explicit expressions for the four-levels occupation probabilities. The analytic treatment explored the properties of coherent oscillations occurred in the atomic excitation processes with intense monochromatic lasers. The conditions under which the population inversion takes place are derived from near-resonant excitations. The criteria to select the basic parameters of pulsed lasers involved in the process are also provided

Comparative investigation of three dose rate meters for their viability in pulsed radiation fields

International Nuclear Information System (INIS)

Gotz, M; Karsch, L; Pawelke, J

2015-01-01

Pulsed radiation fields, characterized by microsecond pulse duration and correspondingly high pulse dose rates, are increasingly used in therapeutic, diagnostic and research applications. Yet, dose rate meters which are used to monitor radiation protection areas or to inspect radiation shielding are mostly designed, characterized and tested for continuous fields and show severe deficiencies in highly pulsed fields. Despite general awareness of the problem, knowledge of the specific limitations of individual instruments is very limited, complicating reliable measurements. We present here the results of testing three commercial dose rate meters, the RamION ionization chamber, the LB 1236-H proportional counter and the 6150AD-b scintillation counter, for their response in pulsed radiation fields of varied pulse dose and duration. Of these three the RamION proved reliable, operating in a pulsed radiation field within its specifications, while the other two instruments were only able to measure very limited pulse doses and pulse dose rates reliably. (paper)

Small compact pulsed electron source for radiation technologies

International Nuclear Information System (INIS)

Korenev, Sergey

2002-01-01

The small compact pulsed electron source for radiation technologies is considered in the report. The electron source consists of pulsed high voltage Marx generator and vacuum diode with explosive emission cathode. The main parameters of electron source are next: kinetic energy is 100-150 keV, beam current is 5-200 A and pulse duration is 100-400 nsec. The distribution of absorbed doses in irradiated materials is considered. The physical feasibility of pulsed low energy electron beam for applications is considered

Intense Ion Pulses for Radiation Effects Research

Science.gov (United States)

2017-04-01

induction linear accelerator that has been developed to deliver intense, up to 50 nC/pulse/mm2, sub-ns pulses of light ions with kinetic energy up to 1.2...II induction linear accelerator for intense ion beam pulses at Berkeley Lab. Figure 3. Helium current and integrated charge versus time at the...under contracts DE-AC02-205CH11231 and DE-AC52-07NA27344. JOURNAL OF RADIATION EFFECTS, Research and Engineering Vol. 35, No. 1, April 2017 158 INTENSE

Radiation from an excited vortex in the Abelian Higgs model

Science.gov (United States)

Arodź, H.; Hadasz, L.

1996-09-01

An excited vortex in the Abelian Higgs model is investigated with the help of a polynomial approximation. The excitation consists of the longitudinal component of a vector field trapped by the vortex. The energy and profile of the excitation as well as its back reaction on the vortex are found in the case of small κ. It turns out that the width of the excited vortex oscillates in time. Moreover, the vector field has a radiative long range component. Also, an upper bound on the amplitude of the excitation is found.

A Radiation Dosimetry Method Using Pulsed Optically Stimulated Luminescence

International Nuclear Information System (INIS)

Akselrod, M.S.; McKeever, S.W.S.

1999-01-01

A method for the determination of absorbed radiation dose is described based on pulsed optically stimulated luminescence (POSL). The method relies upon the stimulation of an irradiated sample with a train of light pulses from a suitable light source (e.g. a laser) using a wavelength which is within the range of wavelengths corresponding to the radiation-induced optical absorption in the irradiated sample. The subsequent emitted light, due to the detrapping of trapped charges and their subsequent recombination with charge of the opposite sign, is synchronously detected in the period between each stimulation pulse. The total luminescence is summed over the desired number of stimulation pulses and this forms the measured POSL signal. By monitoring the emitted light only in the period between stimulation pulses one can reduce the optical filtering required to discriminate between the stimulation light and the emission light; in this way a high measurement efficiency, and, therefore, a high radiation sensitivity (luminescence intensity per unit absorbed dose) is achieved. Key parameters in the method are the intrinsic luminescence lifetime for the material being used as the luminescent detector, the width of the optical stimulation pulse, and the period between pulses. For optimum operation the measurement parameters should be such that both the pulse width and the time between pulses are much less than the luminescence lifetime. By appropriate choice of the power of the optical stimulation, the frequency of the stimulation pulses, and the total stimulation period, one can also re-measure the absorbed dose several times. In this way, a re-read capability is available with the procedure. The method is illustrated using light from a 2nd-harmonic Nd:YAG laser, with irradiated, anion-deficient aluminium oxide as the luminescent detector material. (author)

Photonuclear excitation of 103Rh by synchrotron radiation

International Nuclear Information System (INIS)

Yoshihara, Kenji; Kaji, Harumi; Sekine, Tsutomu; Mukoyama, Takeshi

1989-01-01

Photonuclear excitation of the 103 Rh nucleus was studied using synchrotron radiation. Formation of the excited state was confirmed by observing K X-rays emitted following the isomeric transition of the 103m Rh with a low-energy photon spectrometer. The intensity of induced activity due to 103 Rh(γ,γ') 103m Rh reaction was determined carefully by subtracting the fluorescent K X-rays due to natural background radiation. The integral cross-section for isomer production of 103m Rh by resonance absorption of photons at 295 keV is found to be (2.1±0.8) x 10 -28 cm 2 eV and is compared with that estimated from the previous experimental value for the 1277-keV level. (author)

Photonuclear excitation of 103Rh by synchrotron radiation

International Nuclear Information System (INIS)

Kaji, Harumi; Yoshihara, Kenji; Mukoyama, Takeshi; Nakajima, Tetsuo

1989-01-01

Photonuclear excitation of 103 Rh nucleus was studied by the use of synchrotron radiation at KEK. Formation of excited state was confirmed by observing Rh K X-rays emitted following the isomeric transition of 103m Rh with a low-energy photon spectrometer. The induced activity due to 103 Rh(γ,γ') 103m Rh reaction was determined carefully by subtracting the fluorescent K X-rays due to natural background radiation. The integral cross-section for 103m Rh by resonance absorption at 295 keV is found to be (1∼2)x10 -28 cm 2 ·eV and is compared with that estimated from the previous experimental value for the 1277-keV level and the calculated value

Achievement of radiative feedback control for long-pulse operation on EAST

Science.gov (United States)

Wu, K.; Yuan, Q. P.; Xiao, B. J.; Wang, L.; Duan, Y. M.; Chen, J. B.; Zheng, X. W.; Liu, X. J.; Zhang, B.; Xu, J. C.; Luo, Z. P.; Zang, Q.; Li, Y. Y.; Feng, W.; Wu, J. H.; Yang, Z. S.; Zhang, L.; Luo, G.-N.; Gong, X. Z.; Hu, L. Q.; Hu, J. S.; Li, J.

2018-05-01

The active feedback control of radiated power to prevent divertor target plates overheating during long-pulse operation has been developed and implemented on EAST. The radiation control algorithm, with impurity seeding via a supersonic molecular beam injection (SMBI) system, has shown great success in both reliability and stability. By seeding a sequence of short neon (Ne) impurity pulses with the SMBI from the outer mid-plane, the radiated power of the bulk plasma can be well controlled, and the duration of radiative control (feedforward and feedback) is 4.5 s during a discharge of 10 s. Reliable control of the total radiated power of bulk plasma has been successfully achieved in long-pulse upper single null (USN) discharges with a tungsten divertor. The achieved control range of {{f}rad} is 20%–30% in L-mode regimes and 18%–36% in H-mode regimes. The temperature of the divertor target plates was maintained at a low level during the radiative control phase. The peak particle flux on the divertor target was decreased by feedforward Ne injection in the L-mode discharges, while the Ne pulses from the SMBI had no influence on the peak particle flux because of the very small injecting volume. It is shown that although the radiated power increased, no serious reduction of plasma-stored energy or confinement was observed during the control phase. The success of the radiation control algorithm and current experiments in radiated power control represents a significant advance for steady-state divertor radiation and heat flux control on EAST for near-future long-pulse operation.

Wave-packet dynamics in alkaline dimers. Investigation and control through coherent excitation with fs-pulses

International Nuclear Information System (INIS)

Sauer, F.N.B.

2007-01-01

During my PhD thesis I investigated alkaline dimers with coherent control in a molecular beam as well as with pump-probe spectroscopy in a magneto-optical trap (MOT). The aim of the coherent control experiments were the isotope selective ionization with phase- and amplitude-shaped fs-pulses. Chapter 4 described the gained results of isotope selective ionization of NaK and KRb in a molecular beam by using different pulse formers. For the NaK dimer was the reached optimization factor R Ph and Ampl 770 =R max /R min =25 between maximization and minimization of the isotopomer ratio ( 23 Na 39 K) + /( 23 Na 41 K) + with phase and amplitude modulation of the fs-pulse with a central wavelength of λ=770 nm. From the electronic ground-state X(1) 1 Σ + ;ν''=0 transfers a one-photon-excitation population in the first excited A(2) 1 Σ + state. The coherent control experiment on KRb was used to maximize and minimize the isotopomer ratio ( 124 KRb) + /( 126 KRb) + . It was the first coherent control experiment with a spectral resolution of 1.84 cm -1 /Pixel. For the phase and amplitude optimization was the received optimization factor between minimization and maximization of the isotopomer ratio R Ph and Ampl =R max /R min =7 at a central wavelength of 840 nm. The results showed a stepwise excitation process from the electronic ground-state in the first excited (2) 1 Σ + state with a further excitation, that is possible over three resonant energy potential curves into the ionic ground-state. In the second part of my thesis I realized pump-probe spectroscopy of Rb 2 dimers in a dark SPOT. (orig.)

Heat effect of pulsed Er:YAG laser radiation

Science.gov (United States)

Hibst, Raimund; Keller, Ulrich

1990-06-01

Pulsed Er:YAG laser radiation has been found to be effective for dental enamel and dentin removal. Damage to the surrounding hard tissue is little, but before testing the Er:YAG laser clinically for the preparation of cavities, possible effects on the soft tissue of the pulp must be known. In order to estimate pulp damage , temperature rise in dentin caused by the laser radiation was measured by a thermocouple. Additionally, temperature distributions were observed by means of a thermal imaging system. The heat effect of a single Er:YAG laser pulse is little and limited to the vicinity of the impact side. Because heat energy is added with each additional pulse , the temperature distribution depends not only on the radiant energy, but also on the number of pulses and the repetition rate. Both irradiation conditions can be found , making irreversible pulp damage either likely or unlikely. The experimental observations can be explained qualitatively by a simple model of the ablation process.

Unveiling the excited state energy transfer pathways in peridinin-chlorophyll a-protein by ultrafast multi-pulse transient absorption spectroscopy.

Science.gov (United States)

Redeckas, Kipras; Voiciuk, Vladislava; Zigmantas, Donatas; Hiller, Roger G; Vengris, Mikas

2017-04-01

Time-resolved multi-pulse methods were applied to investigate the excited state dynamics, the interstate couplings, and the excited state energy transfer pathways between the light-harvesting pigments in peridinin-chlorophyll a-protein (PCP). The utilized pump-dump-probe techniques are based on perturbation of the regular PCP energy transfer pathway. The PCP complexes were initially excited with an ultrashort pulse, resonant to the S 0 →S 2 transition of the carotenoid peridinin. A portion of the peridinin-based emissive intramolecular charge transfer (ICT) state was then depopulated by applying an ultrashort NIR pulse that perturbed the interaction between S 1 and ICT states and the energy flow from the carotenoids to the chlorophylls. The presented data indicate that the peridinin S 1 and ICT states are spectrally distinct and coexist in an excited state equilibrium in the PCP complex. Moreover, numeric analysis of the experimental data asserts ICT→Chl-a as the main energy transfer pathway in the photoexcited PCP systems. Copyright © 2017 Elsevier B.V. All rights reserved.

Control of giant pulse duration in neodymium mini lasers with controllable cavity length and pulsed pumping

International Nuclear Information System (INIS)

Berenberg, Vladimir A.; Cervantes, Miguel A.; Terpugov, Vladimir S.

2006-01-01

In a solid-state laser incident on aLiNdP4O12 crystal, pumped by a short light pulse, giant pulse oscillation without the use of resonator Q switching is realized. Tuning of the oscillation pulse duration from 2 up to 20 ns is achieved by changing the cavity length from 24 to 3 mm, respectively. Our analysis of this mode of laser radiation is made on the basis of the rate equations. The factors influencing oscillation pulse duration a reinvestigated. It is shown that in a limiting case the minimal value of the pulse duration is limited by only the rate of excitation transfer from the pumping band to the metastable level

Multiple excitation regenerative amplifier inertial confinement system

International Nuclear Information System (INIS)

George, V.E.; Haas, R.A.; Krupke, W.F.; Schlitt, L.G.

1980-01-01

The invention relates to apparatus and methods for producing high intensity laser radiation generation which is achieved through an optical amplifier-storage ring design. One or two synchronized, counterpropagating laser pulses are injected into a regenerative amplifier cavity and amplified by gain media which are pumped repetitively by electrical or optical means. The gain media excitation pulses are tailored to efficiently amplify the laser pulses during each transit. After the laser pulses have been amplified to the desired intensity level, they are either switched out of the cavity by some switch means, as for example an electro-optical device, for any well known laser end uses, or a target means may be injected into the regenerative amplifier cavity in such a way as to intercept simultaneously the counterpropagating laser pulses. One such well known end uses to which this invention is intended is for production of high density and temperature plasmas suitable for generating neutrons, ions and x-rays and for studying matter heated by high intensity laser radiation

Radiation from an excited vortex in the Abelian Higgs model

International Nuclear Information System (INIS)

Arodz, H.; Hadasz, L.

1996-01-01

An excited vortex in the Abelian Higgs model is investigated with the help of a polynomial approximation. The excitation consists of the longitudinal component of a vector field trapped by the vortex. The energy and profile of the excitation as well as its back reaction on the vortex are found in the case of small κ. It turns out that the width of the excited vortex oscillates in time. Moreover, the vector field has a radiative long range component. Also, an upper bound on the amplitude of the excitation is found. copyright 1996 The American Physical Society

Generating high-power short terahertz electromagnetic pulses with a multifoil radiator.

Science.gov (United States)

Vinokurov, Nikolay A; Jeong, Young Uk

2013-02-08

We describe a multifoil cone radiator capable of generating high-field short terahertz pulses using short electron bunches. Round flat conducting foil plates with successively decreasing radii are stacked, forming a truncated cone with the z axis. The gaps between the foil plates are equal and filled with some dielectric (or vacuum). A short relativistic electron bunch propagates along the z axis. At sufficiently high particle energy, the energy losses and multiple scattering do not change the bunch shape significantly. When passing by each gap between the foil plates, the electron bunch emits some energy into the gap. Then, the radiation pulses propagate radially outward. For transverse electromagnetic waves with a longitudinal (along the z axis) electric field and an azimuthal magnetic field, there is no dispersion in these radial lines; therefore, the radiation pulses conserve their shapes (time dependence). At the outer surface of the cone, we have synchronous circular radiators. Their radiation field forms a conical wave. Ultrashort terahertz pulses with gigawatt-level peak power can be generated with this device.

Picosecond, single pulse electron linear accelerator

International Nuclear Information System (INIS)

Kikuchi, Riichi; Kawanishi, Masaharu

1979-01-01

The picosecond, single pulse electron linear accelerators, are described, which were installed in the Nuclear Engineering Laboratory of the University of Tokyo and in the Nuclear Radiation Laboratory of the Osaka University. The purpose of the picosecond, single pulse electron linear accelerators is to investigate the very short time reaction of the substances, into which gamma ray or electron beam enters. When the electrons in substances receive radiation energy, the electrons get high kinetic energy, and the energy and the electric charge shift, at last to the quasi-stable state. This transient state can be experimented with these special accelerators very accurately, during picoseconds, raising the accuracy of the time of incidence of radiation and also raising the accuracy of observation time. The outline of these picosecond, single pulse electron linear accelerators of the University of Tokyo and the Osaka University, including the history, the systems and components and the output beam characteristics, are explained. For example, the maximum energy 30 -- 35 MeV, the peak current 1 -- 8 n C, the pulse width 18 -- 40 ps, the pulse repetition rate 200 -- 720 pps, the energy spectrum 1 -- 1.8% and the output beam diameter 2 -- 5 mm are shown as the output beam characteristics of the accelerators in both universities. The investigations utilizing the picosecond single pulse electron linear accelerators, such as the investigation of short life excitation state by pulsed radiation, the dosimetry study of pulsed radiation, and the investigation of the transforming mechanism and the development of the transforming technology from picosecond, single pulse electron beam to X ray, vacuum ultraviolet ray and visual ray, are described. (Nakai, Y.)

Use of a 3-MV proton accelerator for study of noble gases, including laser ionization of excited states

International Nuclear Information System (INIS)

Hurst, G.S.; Judish, J.P.; Nayfeh, M.H.; Parks, J.E.; Payne, M.G.; Wagner, E.B.

1974-01-01

The use of a pulsed 3-MV accelerator to study energy pathways in the noble gases is described. The objectives of pathways research are to obtain (1) information on the spectrum of excited states produced by a charged particle in a noble gas, (2) the rate of decay of the various states through various channels as a function of gas pressure, and (3) the modification of the decay channels due to the introduction of foreign species. A new energy pathways model is presented for helium as a general illustration. A method for the study of excited states, using a laser ionization technique is reported. Use is made of a laser which is tuned to a resonance transition between the desired excited state and some higher excited state. Photons in the same pulse photoionize the higher excited state; thus the ionization current vs photon wavelength has a resonance structure. Absolute yields of selected excited states can be obtained whenever the photon fluence per pulse is large enough to saturate the ionization current. A general summary is given of experimental facilities which include a 3-MV Van de Graaff accelerator, electronics for measuring radiation lifetimes, vacuum ultraviolet spectrometers, and a pulsed laser facility for direct study of excited states. Finally, the relevance of pathways research to (1) the interaction of radiation with matter, (2) the development of gas lasers, and (3) methods of ultrasensitive elemental analysis is pointed out

Simulation of the saturation curve of the ionization chamber in overlapping pulsed radiation

International Nuclear Information System (INIS)

Park, Se Hwan; Kim, Yong Kyun; Kim, Han Soo; Kang, Sang Mook; Ha, Jang Ho

2006-01-01

Procedures for determination of collection efficiency in ionization chambers have been studied by numerous investigators. If the theoretical approach for air-filled ionization chambers exposed to continuous radiation is considered, the result in the near-saturation region is a linear relationship between ) (1/I(V) vs 1/V 2 , where I(V) is the current measured with the ionization chamber at a given polarization voltage V . For pulsed radiation beams, Boag developed a model and the resulted in a linear relationship between ) (1/I(V) and 1/V when the collection efficiency, f , is larger than 0.9. The assumption of the linear relationship of ) (1/I(V) with 1/V or 1/V 2 in the near-saturation region makes the determination of the saturation current simple, since the linear relationship may be determined with only two measured data points. The above discussion of the collection efficiency of the ionization chamber exposed to the pulsed radiation is valid only if each pulse is cleared before the next one occurs. The transit times of the ions in the chamber must be shorter than the time interval between the radiation pulses. Most of the previous works concerning the characteristics of the saturation curve of an ionization chamber in the pulsed beam were done for the case where the transit times of the ions were shorter than the interval between the radiation pulses. However, the experimental data for the intermediate case, where the ion transit time was comparable to the interval between the radiation pulses or the ion transit time was slightly longer than the interval between the radiation pulses, were rare. The saturation curves of the ionization chambers in the pulsed radiation were measured with the pulse beamed electron accelerator at the Korea Atomic Energy Research Institute (KAERI), where the ion transit times in the ionization chambers were longer than the time interval between the radiation pulses. We used two ionization chambers: one was a commercial thimble

Radiation damage in nonmetallic solids under dense electronic excitation

International Nuclear Information System (INIS)

Itoh, Noriaki; Tanimura, Katsumi; Nakai, Yasuo

1992-01-01

Basic processes of radiation damage of insulators by dense electronic excitation are reviewed. First it is pointed out that electronic excitation of nonmetallic solids produces the self-trapped excitons and defect-related metastable states having relatively long lifetimes, and that the excitation of these metastable states, produces stable defects. The effects of irradiation with heavy ions, including track registration, are surveyed on the basis of the microscopic studies. It is pointed out also that the excitation of the metastable states plays a role in laser-induced damage at relatively low fluences, while the laser damage has been reported to be governed by heating of free electrons produced by multiphoton excitation. Difference in the contributions of the excitation of metastable defects to laser-induced damage of surfaces, or laser ablation, and laser-induced bulk damage is stressed. (orig.)

Radiative and Excited State Charmonium Physics

Energy Technology Data Exchange (ETDEWEB)

Jozef Dudek

2007-07-30

Renewed interest in the spectroscopy of charmonium has arisen from recent unexpected observations at $e^+e^-$ colliders. Here we report on a series of works from the previous two years examining the radiative physics of charmonium states as well as the mass spectrum of states of higher spin and internal excitation. Using new techniques applied to Domain-Wall and Clover quark actions on quenched isotropic and anisotropic lattices, radiative transitions and two-photon decays are considered for the first time. Comparisons are made with experimental results and with model approaches. Forthcoming application to the light-quark sector of relevance to experiments like Jefferson Lab's GlueX is discussed.

ARTICLES: Thermohydrodynamic models of the interaction of pulse-periodic radiation with matter

Science.gov (United States)

Arutyunyan, R. V.; Baranov, V. Yu; Bol'shov, Leonid A.; Malyuta, D. D.; Mezhevov, V. S.; Pis'mennyĭ, V. D.

1987-02-01

Experimental and theoretical investigations were made of the processes of drilling and deep melting of metals by pulsed and pulse-periodic laser radiation. Direct photography of the surface revealed molten metal splashing due to interaction with single CO2 laser pulses. A proposed thermohydrodynamic model was used to account for the experimental results and to calculate the optimal parameters of pulse-periodic radiation needed for deep melting. The melt splashing processes were simulated numerically.

Utilizations of intense pulsed neutron source in radiochemistry and radiation chemistry

International Nuclear Information System (INIS)

Shiokawa, Takanobu; Yoshihara, Kenji; Kaji, Harumi; Kusaka, Yuzuru; Tabata, Yoneho.

1975-01-01

Intense pulsed neutron sources is expected to supply more useful and fundamental informations in radiochemistry and radiation chemistry. Short-lived intermediate species may be detected and the mechanisms of radiation induced reactions will be elucidated more precisely. Analytical application of pulsed neutrons is also very useful. (auth.)

Impact of ultrafast demagnetization process on magnetization reversal in L10 FePt revealed using double laser pulse excitation

Science.gov (United States)

Shi, J. Y.; Tang, M.; Zhang, Z.; Ma, L.; Sun, L.; Zhou, C.; Hu, X. F.; Zheng, Z.; Shen, L. Q.; Zhou, S. M.; Wu, Y. Z.; Chen, L. Y.; Zhao, H. B.

2018-02-01

Ultrafast laser induced magnetization reversal in L10 FePt films with high perpendicular magnetic anisotropy was investigated using single- and double-pulse excitations. Single-pulse excitation beyond 10 mJ cm-2 caused magnetization (M) reversal at the applied fields much smaller than the static coercivity of the films. For double-pulse excitation, both coercivity reduction and reversal percentage showed a rapid and large decrease with the increasing time interval (Δt) of the two pulses in the range of 0-2 ps. In this Δt range, the maximum demagnetization (ΔMp) was also strongly attenuated, whereas the integrated demagnetization signals over more than 10 ps, corresponding to the average lattice heat effect, showed little change. These results indicate that laser induced M reversal in FePt films critically relies on ΔMp. Because ΔMp is determined by spin temperature, which is higher than lattice temperature, utilizing an ultrafast laser instead of a continuous-wave laser in laser-assisted M reversal may reduce the overall deposited energy and increase the speed of recording. The effective control of M reversal by slightly tuning the time delay of two laser pulses may also be useful for ultrafast spin manipulation.

Excitation of intense shock waves by soft X-radiation

Energy Technology Data Exchange (ETDEWEB)

Branitskij, A V; Fortov, V E; Danilenko, K N; Dyabilin, K S; Grabovskij, E V; Vorobev, O Yu; Lebedev, M E; Smirnov, V P; Zakharov, A E; Persyantsev, I V [Troitsk Inst. of Innovative and Fusion Research, Troitsk (Russian Federation)

1997-12-31

Investigation of the shock waves generated by soft x radiation in Al, Sn, Fe, and Pb targets is reported. The soft x radiation was induced by the dynamic compression and heating of the cylindrical z-pinch plasma generated in the ANGARA-5-1 pulsed power machine. The temperature of the z-pinch plasma was as high as 60 - 120 eV, and the duration of the x-ray pulse reached 30 ns FWHM. Thick stepped Al/Pb, Sn/Pb, and pure Pb targets were used. The results of experiments show that uniform intense shock waves can be generated by z-pinch plasma soft x-ray radiation. The uniformity of the shock is very high. At a flux power of the order of several TW/cm{sup 2}, a shock pressure of some hundreds of GPa was achieved. (J.U.). 3 figs., 11 refs.

Excitation of intense shock waves by soft X-radiation

International Nuclear Information System (INIS)

Branitskij, A.V.; Fortov, V.E.; Danilenko, K.N.; Dyabilin, K.S.; Grabovskij, E.V.; Vorobev, O. Yu.; Lebedev, M.E.; Smirnov, V.P.; Zakharov, A.E.; Persyantsev, I.V.

1996-01-01

Investigation of the shock waves generated by soft x radiation in Al, Sn, Fe, and Pb targets is reported. The soft x radiation was induced by the dynamic compression and heating of the cylindrical z-pinch plasma generated in the ANGARA-5-1 pulsed power machine. The temperature of the z-pinch plasma was as high as 60 - 120 eV, and the duration of the x-ray pulse reached 30 ns FWHM. Thick stepped Al/Pb, Sn/Pb, and pure Pb targets were used. The results of experiments show that uniform intense shock waves can be generated by z-pinch plasma soft x-ray radiation. The uniformity of the shock is very high. At a flux power of the order of several TW/cm 2 , a shock pressure of some hundreds of GPa was achieved. (J.U.). 3 figs., 11 refs

Method to generate a pulse train of few-cycle coherent radiation

Directory of Open Access Journals (Sweden)

Bryant Garcia

2016-09-01

Full Text Available We develop a method to generate a long pulse train of few-cycle coherent radiation by modulating an electron beam with a high power laser. The large energy modulation disperses the beam in a radiating undulator and leads to the production of phase-locked few-cycle coherent radiation pulses. These pulses are produced at a high harmonic of the modulating laser, and are longitudinally separated by the modulating laser wavelength. We discuss an analytical model for this scheme and investigate the temporal and spectral properties of this radiation. This model is compared with numerical simulation results using the unaveraged code Puffin. We examine various harmful effects and how they might be avoided, as well as a possible experimental realization of this scheme.

Application of pulse spectro- zonal luminescent method for the rapid method of material analysis

International Nuclear Information System (INIS)

Lisitsin, V.M.; Oleshko, V.I.; Yakovlev, A.N.

2004-01-01

Full text: The scope of luminescent methods of the analysis covers enough a big around of substances as the luminescence can be excited in overwhelming majority of nonmetals. Analytical opportunities of luminescent methods can be essentially expanded by use of pulse excitation and registration of spectra of a luminescence with the time resolved methods. The most perspective method is to use pulses of high-current electron beams with the nanosecond duration for excitation from the following reasons: excitation is carried out ionizing, deeply enough by a penetrating radiation; the pulse of radiation has high capacity, up to 10 8 W, but energy no more than 1 J; the pulse of radiation has the nanosecond duration. Electrons with energy in 300-400 keV will penetrate on depth into some tenth shares of mm, i.e. they create volumetric excitation of a sample. Therefore the luminescence raised by an electronic beam has the information about volumetric properties of substance. High density of excitation allow to find out and study the centers (defects) having a small yield of a luminescence, to analyze the weakly luminescent objects. Occurrence of the new effects is possible useful to analyze of materials. There is an opportunity of reception of the information from change of spectral structure of a luminescence during the time after the ending of a pulse of excitation and kinetic characteristics of attenuation of luminescence. The matter is the energy of radiation is absorbed mainly by a matrix, then electronic excitations one is transferred the centers of a luminescence (defects) of a lattice. Therefore during the time after creation electronic excitations the spectrum of a luminescence can repeatedly change, transferring the information on the centers (defects) which are the most effective radiators at present time. Hence, the study of change of spectra of radiation during the time allows providing an additional way of discrimination of the information on the centers of a

Sound Radiation of Aerodynamically Excited Flat Plates into Cavities

Directory of Open Access Journals (Sweden)

Johannes Osterziel

2017-10-01

Full Text Available Flow-induced vibrations and the sound radiation of flexible plate structures of different thickness mounted in a rigid plate are experimentally investigated. Therefore, flow properties and turbulent boundary layer parameters are determined through measurements with a hot-wire anemometer in an aeroacoustic wind tunnel. Furthermore, the excitation of the vibrating plate is examined by laser scanning vibrometry. To describe the sound radiation and the sound transmission of the flexible aluminium plates into cavities, a cuboid-shaped room with adjustable volume and 34 flush-mounted microphones is installed at the non flow-excited side of the aluminium plates. Results showed that the sound field inside the cavity is on the one hand dependent on the flow parameters and the plate thickness and on the other hand on the cavity volume which indirectly influences the level and the distribution of the sound pressure behind the flexible plate through different excited modes.

Enhancement of nonlinear optical response of weakly confined excitons in GaAs thin films by spectrally rectangle-shape-pulse-excitation

International Nuclear Information System (INIS)

Kojima, O; Isu, T; Ishi-Hayase, J; Sasaki, M; Tsuchiya, M

2007-01-01

We report the enhancement of the nonlinear optical response of the weakly confined excitons with use of spectrally rectangular pulse. The nonlinear optical response was investigated as a function of excitation energy by a degenerate four-wave-mixing (DFWM) technique. In the case that the laser pulse with the controlled spectral shape excites the plural exciton states simultaneously, the DFWM signal intensity is enhanced by a factor of two in comparison with the intensity under the excitation of a single exciton state. This enhancement is caused by the superposition of the nonlinear optical responses from the plural exciton states

Multi-Pulse Excitation for Underwater Analysis of Copper-Based Alloys Using a Novel Remote Laser-Induced Breakdown Spectroscopy (LIBS) System.

Science.gov (United States)

Guirado, Salvador; Fortes, Francisco J; Laserna, J Javier

2016-04-01

In this work, the use of multi-pulse excitation has been evaluated as an effective solution to mitigate the preferential ablation of the most volatile elements, namely Sn, Pb, and Zn, observed during laser-induced breakdown spectroscopy (LIBS) analysis of copper-based alloys. The novel remote LIBS prototype used in this experiments featured both single-pulse (SP-LIBS) and multi-pulse excitation (MP-LIBS). The remote instrument is capable of performing chemical analysis of submersed materials up to a depth of 50 m. Laser-induced breakdown spectroscopy analysis was performed at air pressure settings simulating the conditions during a real subsea analysis. A set of five certified bronze standards with variable concentration of Cu, As, Sn, Pb, and Zn were used. In SP-LIBS, signal emission is strongly sensitive to ambient pressure. In this case, fractionation effect was observed. Multi-pulse excitation circumvents the effect of pressure over the quantitative analysis, thus avoiding the fractionation phenomena observed in single pulse LIBS. The use of copper as internal standard minimizes matrix effects and discrepancies due to variation in ablated mass. © The Author(s) 2016.

Efficient excitation of nonlinear phonons via chirped pulses: Induced structural phase transitions

Science.gov (United States)

Itin, A. P.; Katsnelson, M. I.

2018-05-01

Nonlinear phononics play important role in strong laser-solid interactions. We discuss a dynamical protocol for efficient phonon excitation, considering recent inspiring proposals: inducing ferroelectricity in paraelectric perovskites, and inducing structural deformations in cuprates [Subedi et al., Phys. Rev. B 89, 220301(R) (2014), 10.1103/PhysRevB.89.220301; Phys. Rev. B 95, 134113 (2017), 10.1103/PhysRevB.95.134113]. High-frequency phonon modes are driven by midinfrared pulses, and coupled to lower-frequency modes those indirect excitations cause structural deformations. We study in more detail the case of KTaO3 without strain, where it was not possible to excite the needed low-frequency phonon mode by resonant driving of the higher frequency one. Behavior of the system is explained using a reduced model of coupled driven nonlinear oscillators. We find a dynamical mechanism which prevents effective excitation at resonance driving. To induce ferroelectricity, we employ driving with sweeping frequency, realizing so-called capture into resonance. The method can be applied to many other related systems.

A novel approach to dual excitation ratiometric optical mapping of cardiac action potentials with di-4-ANEPPS using pulsed LED excitation.

Science.gov (United States)

Bachtel, Andrew D; Gray, Richard A; Stohlman, Jayna M; Bourgeois, Elliot B; Pollard, Andrew E; Rogers, Jack M

2011-07-01

We developed a new method for ratiometric optical mapping of transmembrane potential (V(m)) in cardiac preparations stained with di-4-ANEPPS. V(m)-dependent shifts of excitation and emission spectra establish two excitation bands (481 nm) that produce fluorescence changes of opposite polarity within a single emission band (575-620 nm). The ratio of these positive and negative fluorescence signals (excitation ratiometry) increases V(m) sensitivity and removes artifacts common to both signals. We pulsed blue (450 ± 10 nm) and cyan (505 ± 15 nm) light emitting diodes (LEDs) at 375 Hz in alternating phase synchronized to a camera (750 frames-per-second). Fluorescence was bandpass filtered (585 ± 20 nm). This produced signals with upright (blue) and inverted (cyan) action potentials (APs) interleaved in sequential frames. In four whole swine hearts with motion chemically arrested, fractional fluorescence for blue, cyan, and ratio signals was 1.2 ± 0.3%, 1.2 ± 0.3%, and 2.4 ± 0.6%, respectively. Signal-to-noise ratios were 4.3 ± 1.4, 4.0 ± 1.2, and 5.8 ± 1.9, respectively. After washing out the electromechanical uncoupling agent, we characterized motion artifact by cross-correlating blue, cyan, and ratio signals with a signal with normal AP morphology. Ratiometry improved cross-correlation coefficients from 0.50 ± 0.48 to 0.81 ± 0.25, but did not cancel all motion artifacts. These findings demonstrate the feasibility of pulsed LED excitation ratiometry in myocardium. © 2011 IEEE

PERCEPTION LEVEL EVALUATION OF RADIO ELECTRONIC MEANS TO A PULSE OF ELECTROMAGNETIC RADIATION

Directory of Open Access Journals (Sweden)

2016-01-01

Full Text Available The method for evaluating the perception level of electronic means to pulsed electromagnetic radiation is consid- ered in this article. The electromagnetic wave penetration mechanism towards the elements of electronic systems and the impact on them are determined by the intensity of the radiation field on the elements of electronic systems. The impact of electromagnetic radiation pulses to the electronic systems refers to physical and analytical parameters of the relationship between exposure to pulses of electromagnetic radiation and the sample parameters of electronic systems. A physical and mathematical model of evaluating the perception level of electronic means to pulsed electromagnetic radiation is given. The developed model was based on the physics of electronics means failure which represents the description of electro- magnetic, electric and thermal processes that lead to the degradation of the original structure of the apparatus elements. The conditions that lead to the total equation electronic systems functional destruction when exposed to electromagnetic radia- tion pulses are described. The internal characteristics of the component elements that respond to the damaging effects are considered. The ratio for the power failure is determined. A thermal breakdown temperature versus pulse duration of expo- sure at various power levels is obtained. The way of evaluation the reliability of electronic systems when exposed to pulses of electromagnetic radiation as a destructive factor is obtained.

Estimation of the contribution of ionization and excitation to the lethal effect of ionizing radiation

International Nuclear Information System (INIS)

Petin, V.G.; Komarov, V.P.

1982-01-01

A simple theoretical model is proposed for estimating the differential contribution of ionization and excitation to the lethal effect of ionizing radiation. Numerical results were obtained on the basis of published experimental data on the ability of bacterial cells Escherichia coli to undergo photoreactivation of radiation-induced damage. It was shown that inactivation by excitation may be highly significant for UV-hypersensitive cells capable of photoreactivation; inactivation by excitation increased with the energy of ionizing radiation and the volume of irradiated suspensions. The data are in qualitative agreement with the assumption of a possible contribution of the UV-component of Cerenkov radiation to the formation of excitations responsible for the lethal effect and the phenomenon of photoreactivation after ionizing radiation. Some predictions from the model are discussed. (orig.)

Measurement of far-infrared subpicosecond coherent radiation for pulse radiolysis

Energy Technology Data Exchange (ETDEWEB)

Kozawa, T. E-mail: kozawa@sanken.osaka-u.ac.jp; Mizutani, Y.; Yokoyama, K.; Okuda, S.; Yoshida, Y.; Tagawa, S

1999-06-01

Using a magnetic bunch compression method, a 26.5 MeV subpicosecond electron single bunch was generated with the L-band linac of Osaka University. The coherent transition radiation emitted from the subpicosecond single bunch was observed at wavelengths from 100 to 700 {mu}m. The intensity was 7.9x10{sup 9} times higher than that of the incoherent transition radiation obtained by calculation. The length of the compressed electron bunch was evaluated to be roughly 50 fs (rms) from the analysis of the spectra of the transition radiation. The coherent transition radiation has high enough intensity to be applied to pulse radiolysis as a pulsed light source.

Development of advanced radiation monitors for pulsed neutron fields

CERN Document Server

AUTHOR|(CDS)2081895

The need of radiation detectors capable of efficiently measuring in pulsed neutron fields is attracting widespread interest since the 60s. The efforts of the scientific community substantially increased in the last decade due to the increasing number of applications in which this radiation field is encountered. This is a major issue especially at particle accelerator facilities, where pulsed neutron fields are present because of beam losses at targets, collimators and beam dumps, and where the correct assessment of the intensity of the neutron fields is fundamental for radiation protection monitoring. LUPIN is a neutron detector that combines an innovative acquisition electronics based on logarithmic amplification of the collected current signal and a special technique used to derive the total number of detected neutron interactions, which has been specifically conceived to work in pulsed neutron fields. Due to its special working principle, it is capable of overcoming the typical saturation issues encountere...

Pulsed laser study of excited states of aromatic molecules absorbed in globular proteins

International Nuclear Information System (INIS)

Cooper, M.; Thomas, J.K.

1977-01-01

Pyrene and several derivatives of pyrene such as pyrene sulfonic acid, and pyrene butyric acid were incorporated into bovine serum albumin (BSA) in aqueous solution. The pyrene chromophore was subsequently excited by a pulse of uv light (lambda = 3471 A) from a Q switched frequency doubled ruby laser. The lifetime of the pyrene excited singlet and triplet states were monitored by time resolved spectrophotometry. Various molecules, such as O 2 and I - , dissolved in the aqueous phase, diffused into the protein and quenched pyrene excited states. The rates of these reactions were followed under a variety of conditions such as pH and temperature and in the presence of inert additives. The rates of pyrene excited-state quenching were often considerably smaller than the rates observed in simple solutions. A comparison of the rates in the protein and homogeneous solutions gives information on the factors such as temperature, charge, and pH that control the movement of small molecules in and into BSA

Origin of the low frequency radiation emitted by radiative polaritons excited by infrared radiation in planar La2O3 films.

Science.gov (United States)

Vincent-Johnson, Anita J; Schwab, Yosyp; Mann, Harkirat S; Francoeur, Mathieu; Hammonds, James S; Scarel, Giovanna

2013-01-23

Upon excitation in thin oxide films by infrared radiation, radiative polaritons are formed with complex angular frequency ω, according to the theory of Kliewer and Fuchs (1966 Phys. Rev. 150 573). We show that radiative polaritons leak radiation with frequency ω(i) to the space surrounding the oxide film. The frequency ω(i) is the imaginary part of ω. The effects of the presence of the radiation leaked out at frequency ω(i) are observed experimentally and numerically in the infrared spectra of La(2)O(3) films on silicon upon excitation by infrared radiation of the 0TH type radiative polariton. The frequency ω(i) is found in the microwave to far infrared region, and depends on the oxide film chemistry and thickness. The presented results might aid in the interpretation of fine structures in infrared and, possibly, optical spectra, and suggest the study of other similar potential sources of electromagnetic radiation in different physical scenarios.

Photoionization and trans-to-cis isomerization of β-cyclodextrin-encapsulated azobenzene induced by two-color two-laser-pulse excitation.

Science.gov (United States)

Takeshita, Tatsuya; Hara, Michihiro

2018-03-15

Azobenzene (1) and the complex resulting from the incorporation of 1 with cyclodextrin (1/CD) are attractive for light-driven applications such as micromachining and chemical biology tools. The highly sensitive photoresponse of 1 is crucial for light-driven applications containing both 1 and 1/CD to reach their full potential. In this study, we investigated the photoionization and trans-to-cis isomerization of 1/CD induced by one- and two-color two-laser pulse excitation. Photoionization of 1/CD, which was induced by stepwise two-photon absorption, was observed using laser pulse excitation at 266nm. Additionally, simultaneous irradiation with 266 and 532nm laser pulses increased the trans-to-cis isomerization yield (Υ t→c ) by 27%. It was concluded that the increase in Υ t→c was caused by the occurrence of trans-to-cis isomerization in the higher-energy singlet state (S n ), which was reached by S 1 →S n transition induced by laser pulse excitation at 532nm. The results of this study are potentially applicable in light-driven applications such as micromachining and chemical biology tools. Copyright © 2018 Elsevier B.V. All rights reserved.

Development of transient collisional excitation x-ray laser with ultra short-pulse laser

International Nuclear Information System (INIS)

Kado, Masataka; Kawachi, Tetsuya; Hasegawa, Noboru; Tanaka, Momoko; Sukegawa, Kouta; Nagashima, Keisuke; Kato, Yoshiaki

2001-01-01

We have observed lasing on Ne-like 3s-3p line from titanium (32.4 nm), Ni-like 4p-4d line from silver (13.9 nm) and tin (11.9 nm) with the transient collisional excitation (TCE) scheme that uses combination of a long pre-pulse (∼ns) and a short main pulse (∼ps). A gain coefficient of 23 cm -1 was measured for plasma length up to 4 mm with silver slab targets. We have also observed lasing on Ne-like and Ni-like lines with new TCE scheme that used pico-seconds laser pulse to generate plasma and observed strong improvement of x-ray laser gain coefficient. A gain coefficient of 14 cm -1 was measured for plasma length up to 6 mm with tin targets. (author)

Vibrational excitation of hydrogen molecules by two-photon absorption and third-harmonic generation

Science.gov (United States)

Miyamoto, Yuki; Hara, Hideaki; Hiraki, Takahiro; Masuda, Takahiko; Sasao, Noboru; Uetake, Satoshi; Yoshimi, Akihiro; Yoshimura, Koji; Yoshimura, Motohiko

2018-01-01

We report the coherent excitation of the vibrational state of hydrogen molecules by two-photon absorption and the resultant third-harmonic generation (THG). Parahydrogen molecules cooled by liquid nitrogen are irradiated by mid-infrared nanosecond pulses at 4.8 μm with a nearly Fourier-transform-limited linewidth. The first excited vibrational state of parahydrogen is populated by two-photon absorption of the mid-infrared photons. Because of the narrow linewidth of the mid-infrared pulses, coherence between the ground and excited states is sufficient to induce higher-order processes. Near-infrared photons from the THG are observed at 1.6 μm. The dependence of the intensity of the near-infrared radiation on mid-infrared pulse energy, target pressure, and cell length is determined. We used a simple formula for THG with consideration of realistic experimental conditions to explain the observed results.

A novel low cost pulse excitation source to study trap spectroscopy of persistent luminescent materials

Science.gov (United States)

Chandrasekhar, Ngangbam; Singh, Nungleppam Monorajan; Gartia, R. K.

2018-04-01

Luminescent techniques require one or the other source of excitations which may vary from high cost X-rays, γ-rays, β-rays etc. to low cost LED. Persistent luminescent materials or Glow-in-the-Dark phosphors are the optical harvesters which store the optical energy from day light illuminating a whole night. They are so sensitive that they can be excited even with the low light of firefly. Therefore, instead of using a high cost excitation source authors have developed a low cost functioning of excitation source controlling short pulses of LED to excite persistent phosphors with the aid of ExpEYES Junior (Hardware/software framework developed by IUAC, New Delhi). Using this, the authors have excited the sample under investigation upto 10 ms. Trap spectroscopy of the pre-excited sample with LED is studied using Thermoluminescence (TL) technique. In this communication, development of the excitation source is discussed and demonstrate the its usefulness in the study of trap spectroscopy of commercially available CaS:Eu2+, Sm3+. Trapping parameters are also evaluated using Computerized Glow Curve Deconvolution (CGCD) technique.

Electronic-excitation induced radiation damage in glasses

Energy Technology Data Exchange (ETDEWEB)

Vigouroux, J P

1985-01-01

In order to understand the microscopic nature of radiation induced defects in insulators, we have studied localization of negative and positive charges in amorphous and monocrystalline SiO2. The behaviour of these charges is linked to creation of point defects by electronic excitation. The role of intense electric fields under irradiation is pointed out.

Losses analysis of soft magnetic ring core under sinusoidal pulse width modulation (SPWM) and space vector pulse width modulation (SVPWM) excitations

Science.gov (United States)

Gao, Hezhe; Li, Yongjian; Wang, Shanming; Zhu, Jianguo; Yang, Qingxin; Zhang, Changgeng; Li, Jingsong

2018-05-01

Practical core losses in electrical machines differ significantly from those experimental results using the standardized measurement method, i.e. Epstein Frame method. In order to obtain a better approximation of the losses in an electrical machine, a simulation method considering sinusoidal pulse width modulation (SPWM) and space vector pulse width modulation (SVPWM) waveforms is proposed. The influence of the pulse width modulation (PWM) parameters on the harmonic components in SPWM and SVPWM is discussed by fast Fourier transform (FFT). Three-level SPWM and SVPWM are analyzed and compared both by simulation and experiment. The core losses of several ring samples magnetized by SPWM, SVPWM and sinusoidal alternating current (AC) are obtained. In addition, the temperature rise of the samples under SPWM, sinusoidal excitation are analyzed and compared.

Self-Resonant Plasma Wake-Field Excitation by a Laser-Pulse with a Steep Leading-Edge for Particle-Acceleration

NARCIS (Netherlands)

Goloviznin, V. V.; van Amersfoort, P. W.

1995-01-01

The self-modulational instability of a relatively long laser pulse with a power close to or less than the critical power for relativistic self-focusing in plasma is considered. Strong wake-field excitation occurs as the result of a correlated transverse and longitudinal evolution of the pulse. The

Radiative lifetime and Lande-factor measurements of the Se I 4p35S 5S2 level using pulsed laser spectroscopy

International Nuclear Information System (INIS)

Zerne, R.

1992-01-01

This diploma project consists of spectroscopic examinations of atomic selenium. Natural selenium was thermally dissociated in a quarts resonance cell keeping the background pressure of selenium molecules low by differential heating. The 4p 3 5S 5 S 2 level was excited by frequency-tripled pulsed dye-laser radiation at 207 nm. From time-resolved recording of the fluorescence decay at 216 nm the natural radiative lifetime of the 5 S 2 level was determined to be 493(15) ns. Quantum-beat and optical double resonance measurements in an external magnetic field yielded g j = 2.0004(10) for the Lande factor

Deep tissue optical imaging of upconverting nanoparticles enabled by exploiting higher intrinsic quantum yield through use of millisecond single pulse excitation with high peak power

DEFF Research Database (Denmark)

Liu, Haichun; Xu, Can T.; Dumlupinar, Gökhan

2013-01-01

We have accomplished deep tissue optical imaging of upconverting nanoparticles at 800 nm, using millisecond single pulse excitation with high peak power. This is achieved by carefully choosing the pulse parameters, derived from time-resolved rate-equation analysis, which result in higher intrinsic...... quantum yield that is utilized by upconverting nanoparticles for generating this near infrared upconversion emission. The pulsed excitation approach thus promises previously unreachable imaging depths and shorter data acquisition times compared with continuous wave excitation, while simultaneously keeping...... therapy and remote activation of biomolecules in deep tissues....

Relaxation and excitation electronic processes in dielectrics irradiated by ultrafast IR and VUV pulses; Processus electroniques d'excitation et de relaxation dans les solides dielectriques excites par des impulsions IR et XUV ultracourtes

Energy Technology Data Exchange (ETDEWEB)

Gaudin, J

2005-11-15

We studied excitation and relaxation of electrons involved during interaction of visible and VUV femtosecond pulses with dielectrics. The generated population of hot electrons, having energy of few eV to few tens of eV above the bottom of the conduction band, is responsible of phenomena ranging to defect creation to optical breakdown. Owing to two techniques: photoemission and transient photoconductivity we improve the understanding of the The first photoemission experiments deal with dielectrics irradiated by 30 fs IR pulses. The photoemission spectra measured show a large population of electrons which energy rise up to 40 eV. We interpret this result in terms of a new absorption process: direct multi-photons inter-branch transitions. The 2. type of photoemission experiments are time resolved 'pump/probe' investigation. We study the relaxation of electrons excited by a VUV pulses. We used the high order harmonics (HOH) as light sources. We found surprisingly long decay time in the range of ps timescale. Last type of experiments is photoconductivity studies of diamond samples. Using HOH as light source we measure the displacement current induced by excited electrons in the conduction band. Those electrons relax mainly by impact ionisation creating secondary electrons. Hence by probing the number of electrons we were able to measure the efficiency of these relaxation processes. We observe a diminution of this efficiency when the energy of exciting photons is above 20 eV. Owing to Monte-Carlo simulation we interpret this result in terms of band structure effect. (author)

Modulation of the electroluminescence emission from ZnO/Si NCs/p-Si light-emitting devices via pulsed excitation

Science.gov (United States)

López-Vidrier, J.; Gutsch, S.; Blázquez, O.; Hiller, D.; Laube, J.; Kaur, R.; Hernández, S.; Garrido, B.; Zacharias, M.

2017-05-01

In this work, the electroluminescence (EL) emission of zinc oxide (ZnO)/Si nanocrystals (NCs)-based light-emitting devices was studied under pulsed electrical excitation. Both Si NCs and deep-level ZnO defects were found to contribute to the observed EL. Symmetric square voltage pulses (50-μs period) were found to notably enhance EL emission by about one order of magnitude. In addition, the control of the pulse parameters (accumulation and inversion times) was found to modify the emission lineshape, long inversion times (i.e., short accumulation times) suppressing ZnO defects contribution. The EL results were discussed in terms of the recombination dynamics taking place within the ZnO/Si NCs heterostructure, suggesting the excitation mechanism of the luminescent centers via a combination of electron impact, bipolar injection, and sequential carrier injection within their respective conduction regimes.

Experimental investigation of 1 GW repeatable ultra-wide band pulse radiating source

International Nuclear Information System (INIS)

Meng Fanbao; Ma Hongge; Zhou Chuanming; Yang Zhoubing; Lu Wei; Ju Bingquan; Yu Huilong

2001-01-01

The single cycle pulse of 1.6 GW peak power with 20 Hz repetition-rate was generated. It radiated a peak power of more than 500 MW with a coaxial biconical antenna. The technological problems of the insulation and energy loss during generating and radiating high peak power ultra-wide band (UWB) pulse have been resolved. The experiments show that the material insulation and dispersion in sub-nanosecond pulse should be investigated deeply

Experimental investigation of 1 GW repeatable ultra-wide band pulse radiating source

Energy Technology Data Exchange (ETDEWEB)

Fanbao, Meng; Hongge, Ma; Chuanming, Zhou; Zhoubing, Yang; Wei, Lu; Bingquan, Ju; Huilong, Yu [China Academy of Engineering Physics, Chengdu (China)

2000-11-01

The single cycle pulse of 1.6 GW peak power with 20 Hz repetition-rate was generated. It radiated a peak power of more than 500 MW with a coaxial biconical antenna. The technological problems of the insulation and energy loss during generating and radiating high peak power ultra-wide band (UWB) pulse have been resolved. The experiments show that the material insulation and dispersion in subnanosecond pulse should be investigated deeply.

Computer modelling of a short-pulse excited dielectric barrier discharge xenon excimer lamp (lambda approx 172 nm)

CERN Document Server

Carman, R J

2003-01-01

A detailed rate-equation analysis has been used to simulate the plasma kinetics in a pulsed-excited dielectric barrier discharge in xenon, under operating conditions where the discharge structure is spatially homogeneous. The one-dimensional model, incorporating 14 species and 70 reaction processes, predicts results that are in good agreement with experimental measurements of the electrical characteristics, and optical (vacuum-ultraviolet (VUV) and visible) pulse shapes. The model reveals that electrical breakdown of the discharge gap occurs via a fast-moving ionization/excitation wavefront that starts close to the anode dielectric and propagates towards the cathode at approx 3x10 sup 5 m s sup - sup 1. The wavefront appears as a result of successive avalanches of electrons that propagate across the discharge gap after release from the cathode dielectric. During breakdown, the mean electron energy in the bulk plasma is close to optimum for preferential excitation of the Xe* 1s sub 4 sub , sub 5 states that fe...

Compression and radiation of high-power short rf pulses. II. A novel antenna array design with combined compressor/radiator elements

KAUST Repository

Sirenko, Kostyantyn

2011-01-01

The paper discusses the radiation of compressed high power short RF pulses using two different types of antennas: (i) A simple monopole antenna and (ii) a novel array design, where each of the elements is constructed by combining a compressor and a radiator. The studies on the monopole antenna demonstrate the possibility of a high power short RF pulse\\'s efficient radiation even using simple antennas. The studies on the novel array design demonstrate that a reduced size array with lower pulse distortion and power decay can be constructed by assembling the array from elements each of which integrates a compressor and a radiator. This design idea can be used with any type of antenna array; in this work it is applied to a phased array.

Features of the mechanoluminescence of thin metal films, excited by short and long laser pulses

International Nuclear Information System (INIS)

Banishev, A.F.; Panchenko, V.Ya.; Shishkov, A.V.

2004-01-01

The results of the study on the deformation-induced luminescence of the fine grain metal films, originating by the impact of the short (submicrosecond) and long (millisecond) laser pulses, are presented. The supposition os made relative to the luminescence excitation mechanism [ru

Cross sections for energy transfer in collisions between two excited sodium atoms

International Nuclear Information System (INIS)

Huennekens, J.; Gallagher, A.

1983-01-01

We have measured cross sections, sigma/sub n/L, for the excitation transfer process Na(3P)+Na(3P)→Na(3S)+Na(nL), where nL is the 4D or 5S level. Our results are sigma/sub 4D/ = 23 A 2 +- 35% and sigma/sub 5S/ = 16 A 2 +- 35% at Tapprox.600 K. To obtain these cross sections we have used pulsed excitation and measured the intensities of 4D, 5S, and 3P fluorescence emissions, and the spatial distribution of excited atoms resulting from radiation diffusion, as well as the excited atom density as a function of time. Additionally, we have accounted for (time-dependent) radiation trapping of 3P and nL level radiation and for the resulting anisotropies of these fluorescence emissions. Comparisons of our results with theory have been made, and their relevance to other experiments is discussed

Confined longitudinal acoustic phonon modes in free-standing Si membranes coherently excited by femtosecond laser pulses

OpenAIRE

Hudert, Florian; Bruchhausen, Axel; Issenmann, Daniel; Schecker, Olivier; Waitz, Reimar; Erbe, Artur; Scheer, Elke; Dekorsy, Thomas; Mlayah, Adnen; Huntzinger, Jean-Roch

2009-01-01

In this Rapid Communication we report the first time-resolved measurements of confined acoustic phonon modes in free-standing Si membranes excited by fs laser pulses. Pump-probe experiments using asynchronous optical sampling reveal the impulsive excitation of discrete acoustic modes up to the 19th harmonic order for membranes of two different thicknesses. The modulation of the membrane thickness is measured with fm resolution. The experimental results are compared with a theoretical model in...

Double discharges in unipolar-pulsed dielectric barrier discharge xenon excimer lamps

International Nuclear Information System (INIS)

Liu Shuhai; Neiger, Manfred

2003-01-01

Excitation of dielectric barrier discharge xenon excimer lamps by unipolar short square pulses is studied in this paper. Two discharges with different polarity are excited by each voltage pulse (double discharge phenomenon). The primary discharge occurs at the top or at the rising flank of the applied unipolar square pulse, which is directly energized by the external circuit. The secondary discharge with the reversed polarity occurs at the falling flank or shortly after the falling flank end (zero external voltage) depending on the pulse width, which is energized by the energy stored by memory charges deposited by the primary discharge. Fast-speed ICCD imaging shows the primary discharge has a conic discharge appearance with a channel broadening on the anode side. This channel broadening increases with increasing the pulse top level. Only the anode-side surface discharge is observed in the primary discharge. The surface discharge on the cathode side which is present in bipolar sine voltage excitation is not observed. On the contrary, the secondary discharge has only the cathode-side surface discharge. The surface discharge on the anode side is not observed. The secondary discharge is much more diffuse than the primary discharge. Time-resolved emission measurement of double discharges show the secondary discharge emits more VUV xenon excimer radiation but less infrared (IR) xenon atomic emission than the primary discharge. It was found that the IR xenon atomic emission from the secondary discharge can be reduced by shortening the pulse width. The energy efficiency of unipolar-pulsed xenon excimer lamps (the overall energy efficiency of double discharges) is much higher than that obtained under bipolar sine wave excitation. The output VUV spectrum under unipolar pulse excitation is found to be identical to that under sine wave excitation and independent of injected electric power

Ionization steps and phase-space metamorphoses in the pulsed microwave ionization of highly excited hydrogen atoms

International Nuclear Information System (INIS)

Bayfield, J.E.; Luie, S.Y.; Perotti, L.C.; Skrzypkowski, M.P.

1996-01-01

As the peak electric field of the microwave pulse is increased, steps in the classical microwave ionization probability of the highly excited hydrogen atom are produced by phase-space metamorphosis. They arise from new layers of Kolmogorov-Arnold-Moser (KAM) islands being exposed as KAM surfaces are destroyed. Both quantum numerical calculations and laboratory experiments exhibit the ionization steps, showing that such metamorphoses influence pulsed semiclassical systems. copyright 1996 The American Physical Society

An ideal scintillator – ZnO:Sc for sub-nanosecond pulsed radiation detection

Energy Technology Data Exchange (ETDEWEB)

Zhang, Kan, E-mail: zhangkan8414@163.com [Northwest Institute of Nuclear Technology, Xi’an 710024 (China); Ouyang, Xiaoping [Northwest Institute of Nuclear Technology, Xi’an 710024 (China); Xi’an Jiaotong University, Xi’an 710049 (China); Song, Zhaohui; Han, Hetong [Northwest Institute of Nuclear Technology, Xi’an 710024 (China); Zuo, Yanbin [China Nonferrous Metal Guilin Research Institute of Geology for Mineral Resource, Guilin 541004 (China); Guan, Xingyin [Northwest Institute of Nuclear Technology, Xi’an 710024 (China); Xi’an Jiaotong University, Xi’an 710049 (China); Tan, Xinjian; Zhang, Zichuan; Liu, Junhong [Northwest Institute of Nuclear Technology, Xi’an 710024 (China)

2014-08-21

ZnO-based scintillators are particularly well suited for use as ultrafast pulsed radiation detectors which have shown broad application prospects in various fields such as the inertial confinement fusion (ICF) diagnosis, the nuclear reaction mechanism, etc. Using the hydro-thermal method, a ZnO single-crystal doped with Scandium (ZnO:Sc) sample was prepared. As a new ZnO-based scintillator, the scintillation characteristics of ZnO:Sc have not been reported previously. In this paper, optical and scintillation characteristics of ZnO:Sc single-crystal were studied. Also a scintillation detector based on ZnO:Sc was designed. Excited by the alpha-particle, the rise time of ZnO:Sc detectors was from 162.5 to 170.7 ps, and the fall time was from 300.4 to 328.8 ps.

An ideal scintillator – ZnO:Sc for sub-nanosecond pulsed radiation detection

International Nuclear Information System (INIS)

Zhang, Kan; Ouyang, Xiaoping; Song, Zhaohui; Han, Hetong; Zuo, Yanbin; Guan, Xingyin; Tan, Xinjian; Zhang, Zichuan; Liu, Junhong

2014-01-01

ZnO-based scintillators are particularly well suited for use as ultrafast pulsed radiation detectors which have shown broad application prospects in various fields such as the inertial confinement fusion (ICF) diagnosis, the nuclear reaction mechanism, etc. Using the hydro-thermal method, a ZnO single-crystal doped with Scandium (ZnO:Sc) sample was prepared. As a new ZnO-based scintillator, the scintillation characteristics of ZnO:Sc have not been reported previously. In this paper, optical and scintillation characteristics of ZnO:Sc single-crystal were studied. Also a scintillation detector based on ZnO:Sc was designed. Excited by the alpha-particle, the rise time of ZnO:Sc detectors was from 162.5 to 170.7 ps, and the fall time was from 300.4 to 328.8 ps

Laser-induced incandescence of suspended particles as a source of excitation of dye luminescence

CERN Document Server

Zelensky, S

2003-01-01

The interaction of pulsed YAG-Nd sup 3 sup + laser radiation with submicron light-absorbing particles suspended in an aqueous solution of Rhodamine 6G is investigated experimentally. The experiments demonstrate that the laser-induced incandescence of suspended particles excites the luminescence of the dissolved dye molecules. The mechanism of the luminescence excitation consists in the reabsorption of the thermal radiation within the volume of the sample cell. On the ground of this mechanism of excitation, a method of measurement of the luminescence quantum yield is proposed and realized. The method requires the knowledge of the geometrical parameters of the cell and does not require the use of reference samples.

An evaluation on environment radiation impact of pulsed reactor

International Nuclear Information System (INIS)

Gao Yingwei; Pu Gongxu; Li Jian

1991-01-01

The dose regulation, assessment scope and assessment method adopted by the environment impact evaluation for the pulsed reactor are discussed. The compute model, the compute programme and the compute result of the dose adopted for the model pulsed reactor are introduced. The probable environment radiation impact under normal status and accident status are also appraised

Laser spectroscopy on atoms and ions using short-wavelength radiation

International Nuclear Information System (INIS)

Larsson, Joergen.

1994-05-01

Radiative properties and energy structures in atoms and ions have been investigated using UV/VUV radiation. In order to obtain radiation at short wavelengths, frequency mixing of pulsed laser radiation in crystals and gases has been performed using recently developed frequency-mixing schemes. To allow the study of radiative lifetimes shorter than the pulses from standard Q-switched lasers, different techniques have been used to obtain sufficiently short pulses. The Hanle effect has been employed following pulsed laser excitation for the same purpose. High-resolution spectroscopic techniques have been adapted for use with the broad-band, pulsed laser sources which are readily available in the UV/VUV spectral region. In order to investigate sources of radiation in the XUV and soft X-ray spectral regions, harmonic generation in rare gases has been studied. The generation of coherent radiation by the interaction between laser radiation and relativistic electrons in a synchrotron storage ring has also been investigated. 60 refs

Red Shift and Broadening of Backward Harmonic Radiation from Electron Oscillations Driven by Femtosecond Laser Pulse

International Nuclear Information System (INIS)

Tian Youwei; Yu Wei; Lu Peixiang; Senecha, Vinod K; Han, Xu; Deng Degang; Li Ruxin; Xu Zhizhan

2006-01-01

The characteristics of backward harmonic radiation due to electron oscillations driven by a linearly polarized fs laser pulse are analysed considering a single electron model. The spectral distributions of the electron's backward harmonic radiation are investigated in detail for different parameters of the driver laser pulse. Higher order harmonic radiations are possible for a sufficiently intense driving laser pulse. We have shown that for a realistic pulsed photon beam, the spectrum of the radiation is red shifted as well as broadened because of changes in the longitudinal velocity of the electrons during the laser pulse. These effects are more pronounced at higher laser intensities giving rise to higher order harmonics that eventually leads to a continuous spectrum. Numerical simulations have further shown that by increasing the laser pulse width the broadening of the high harmonic radiations can be controlled

Research of pulse gamma ray radiation effect on microcontroller system

International Nuclear Information System (INIS)

Yang Shanchao; Ma Qiang; Jin Xiaoming; Li Ruibin; Lin Dongsheng; Chen Wei; Liu Yan

2012-01-01

An experimental result of power chip LM7805 and microcontroller EE80C196KC20 based on the EE80C196KC20 testing system was presented. The pulse gamma ray radiation effect was investigated using 'Qiangguang-Ⅰ' accelerator. Latchup threshold of the microcontroller was obtained, and the relationship of supply current and I/O output with the transient dose rate was observed. The result shows that the restrainability of power chip on pulse gamma ray radiation induces microcontroller latchup effect. (authors)

Coherent Smith-Purcell radiation as a pulse length diagnostic

International Nuclear Information System (INIS)

Lampel, M.C.

1997-01-01

Recently, Smith-Purcell radiation has been studied as a candidate for laser-type radiation production in the submillimeter regime. With appropriate choices of beam energy, impact parameter, and grating spacing, there is good coupling to strongly polarized, forward directed radiation. Another regime of possible interest is to use Smith-Purcell radiation as a pulse length diagnostic for medium to high energy electron beams of extremely short pulse duration, on the order of tens of femtoseconds to 1000 fs. Strongly in favor of development of such a diagnostic is its relatively non-destructive nature. With the electron beam passing near, but not through, a metal grating, reaction of the beam distribution itself to the production of the radiation is reduced relative to the much stronger scattering induced by passage through a foil. By careful choice of parameters usable diagnostic radiation ought to be produced with acceptably small emittance growth for an on-line beam monitor, even for the extremely bright electron beams proposed for X-ray FELs, Compton backscatter X-ray sources, or laser/plasma accelerator schemes. In this paper coherent and incoherent Smith-Purcell radiation is examined for reasonable operating parameters of the SATURNUS system at UCLA, with comparisons with results reported from the accelerator test facility (ATF) at Brookhaven National Laboratory. (orig.)

Combination transition radiation in a medium excited by an electromagnetic field

International Nuclear Information System (INIS)

Kalashnikova, Yu.S.

1976-01-01

The radiation emitted by a uniformly moving charged particle in a medium excited by an electromagnetic field is considered by taking into account the interaction between the electromagnetic waves and optical phonon wave. The frequencies are found, in the vicinity of which the two-wave approximation should be applied in order to determine the radiation field. It is shown that in the vicinity of these frequencies the radiation considerably differs from the Cherenkov radiation

Chirped or time modulated excitation compared to short pulses for photoacoustic imaging in acoustic attenuating media

Science.gov (United States)

Burgholzer, P.; Motz, C.; Lang, O.; Berer, T.; Huemer, M.

2018-02-01

In photoacoustic imaging, optically generated acoustic waves transport the information about embedded structures to the sample surface. Usually, short laser pulses are used for the acoustic excitation. Acoustic attenuation increases for higher frequencies, which reduces the bandwidth and limits the spatial resolution. One could think of more efficient waveforms than single short pulses, such as pseudo noise codes, chirped, or harmonic excitation, which could enable a higher information-transfer from the samples interior to its surface by acoustic waves. We used a linear state space model to discretize the wave equation, such as the Stoke's equation, but this method could be used for any other linear wave equation. Linear estimators and a non-linear function inversion were applied to the measured surface data, for onedimensional image reconstruction. The proposed estimation method allows optimizing the temporal modulation of the excitation laser such that the accuracy and spatial resolution of the reconstructed image is maximized. We have restricted ourselves to one-dimensional models, as for higher dimensions the one-dimensional reconstruction, which corresponds to the acoustic wave without attenuation, can be used as input for any ultrasound imaging method, such as back-projection or time-reversal method.

On the biphoton excitation of the fluorescence of the bacteriochlorophyll molecules of purple photosynthetic bacteria by powerful near IR femto-picosecond pulses

Energy Technology Data Exchange (ETDEWEB)

Borisov, A. Yu., E-mail: borissov@belozersky.msu.ru [Moscow State University, Belozersky Institute of Physicochemical Biology (Russian Federation)

2011-11-15

The authors of a number of experimental works detected nonresonance biphoton excitation of bacteriochlorophyll molecules, which represent the main pigment in the light-absorbing natural 'antenna' complexes of photosynthesizing purple bacteria, by femtosecond IR pulses (1250-1500 nm). They believe that IR quanta excite hypothetic forbidden levels of the pigments of these bacteria in the double frequency range 625-750 nm. We propose and ground an alternative triplet mechanism to describe this phenomenon. According to our hypothesis, the mechanism of biphoton excitation of molecules by IR quanta can manifest itself specifically, through high triplet levels of molecules in the high fields induced by femtosecond-picosecond laser pulses.

Ultraviolet germicidal efficacy as a function of pulsed radiation parameters studied by spore film dosimetry.

Science.gov (United States)

Bauer, Stefan; Holtschmidt, Hans; Ott, Günter

2018-01-01

Disinfection by pulsed ultraviolet (UV) radiation is a commonly used method, e.g. in industry or medicine and can be carried out either with lasers or broadband UV radiation sources. Detrimental effects to biological materials depending on parameters such as pulse duration τ or pulse repetition frequency f p are well-understood for pulsed coherent UV radiation, however, relatively little is known for its incoherent variant. Therefore, within this work, it is the first time that disinfection rates of pulsed and continuous (cw) incoherent UV radiation studied by means of spore film dosimetry are presented, compared with each other, and in a second step further investigated regarding two pulse parameters. After analyzing the dynamic range of the Bacillus subtilis spore films with variable cw radiant exposures H=5-100Jm -2 a validation of the Bunsen-Roscoe law revealed its restricted applicability and a 28% enhanced detrimental effect of pulsed compared to cw incoherent UV radiation. A radiant exposure H=50Jm -2 and an irradiance E=0.5Wm -2 were found to be suitable parameters for an analysis of the disinfection rate as a function of τ=0.5-10ms and f p =25-500Hz unveiling that shorter pulses and lower frequencies inactivate more spores. Finally, the number of applied pulses as well as the experiment time were considered with regard to spore film disinfection. Copyright © 2017 Elsevier B.V. All rights reserved.

Excitation and deexcitation of the Si-H stretching mode in a Si:H with picosecond free electron laser pulses

International Nuclear Information System (INIS)

Xu, Z.; Fauchet, M.; Rella, C.W.

1995-01-01

Hydrogen in amorphous and crystalline silicon has been the topic of intense theoretical and experimental investigations for more than one decade. To better understand how the Si-H bonds interact with the Si matrix and how they can be broken, it would be useful to excite selectively these bonds and monitor the energy flow from the Si-H bonds into the bulk Si modes. One attractive way of exciting the Si-H modes selectively is with an infrared laser tuned to a Si-H vibrational mode. Unfortunately, up to now, this type of experiment had not been possible because of the lack of a laser producing intense, ultrashort pulses that are tunable in the mid infrared. In this presentation, we report the first measurement where a 1 picosecond long laser pulse was used to excite the Si-H stretching modes near 2000 cm -1 and another identical laser pulse was used to measure the deexcitation from that specific vibrational mode. The laser was the Stanford free electron laser generating ∼1 ps-long pulses, tunable in the 5 μm region and focussed to an intensity of ∼1 GW/cm 2 . The pump-probe measurements were performed in transmission at room temperature on several 2 μm thick a-Si:H films deposited on c-Si. Samples with predominant Si-H 1 modes, predominant Si-H n>1 modes and with a mixture of modes were prepared. The laser was tuned on resonance with either of these modes. Immediately after excitation, we observe a bleaching of the infrared absorption, which can be attributed to excitation of the Si-H mode. Beaching is expected since, as a result of anharmonicity, the detuning between the (E 3 - E 2 ) resonance and the (E 2 - E 1 ) resonance is larger than the laser bandwidth. Note that despite the anharmonicity, it should be possible to climb the vibrational ladder due to power broadening

Deconvolving the temporal response of photoelectric x-ray detectors for the diagnosis of pulsed radiations

International Nuclear Information System (INIS)

Zou, Shiyang; Song, Peng; Pei, Wenbing; Guo, Liang

2013-01-01

Based on the conjugate gradient method, a simple algorithm is presented for deconvolving the temporal response of photoelectric x-ray detectors (XRDs) to reconstruct the resolved time-dependent x-ray fluxes. With this algorithm, we have studied the impact of temporal response of XRD on the radiation diagnosis of hohlraum heated by a short intense laser pulse. It is found that the limiting temporal response of XRD not only postpones the rising edge and peak position of x-ray pulses but also smoothes the possible fluctuations of radiation fluxes. Without a proper consideration of the temporal response of XRD, the measured radiation flux can be largely misinterpreted for radiation pulses of a hohlraum heated by short or shaped laser pulses

Pulsed radiation studies of carotenoid radicals and excited states

International Nuclear Information System (INIS)

Burke, M.

2001-04-01

The one-electron reduction potentials of the radical cations of five dietary carotenoids, in aqueous micellar environments, have been obtained from a pulse radiolysis study of electron transfer between the carotenoids and tryptophan radical cations as a function of pH, and lie in the range 980 to 1060 mV. The decays of the carotenoid radical cations suggest a distribution of exponential lifetimes. The radicals persist for up to about one second, depending on the medium and may re-orientate within a biological environment to react with other biomolecules, such as tyrosine, cysteine or ascorbic acid, which was indeed confirmed. Spectral information of carotenoid pigmented liposomes has been collected, subsequently pulse radiolysis was used to generate the radical cations of β-carotene, zeaxanthin and lutein, in unilamellar vesicles of dipalmitoyl phosphatidyl choline. The rate constants for the 'repair' of these carotenoid radical cations by water-soluble vitamin C were found to be similar (∼1 x 10 7 M -1 s -1 ) for β-carotene and zeaxanthin and somewhat lower (∼0.5 x 10 7 M -1 s -1 ) for lutein. The results are discussed in terms of the microenvironment of the carotenoids and suggest that for β-carotene, a hydrocarbon carotenoid, the radical cation is able to interact with a water-soluble species even though the parent hydrocarbon carotenoid is probably entirely in the non-polar region of the liposome. Studies investigating the ability of ingested lycopene to protect human lymphoid cells against singlet oxygen and nitrogen dioxide radical mediated cell damage have shown that a high lycopene diet is beneficial in protecting human cells against reactive oxygen species. Triplet states of carotenoids were produced in benzene solvent and their triplet lifetimes were found to depend on the concentration of the parent molecule. The rate constants obtained for ground state quenching correlate with the number of conjugated double bonds, the longer chain systems having

Peculiarities of biological effect of pulsed laser radiation and 60Co γ rays on microorganisms

International Nuclear Information System (INIS)

Petin, V.G.; Rusina, L.K.; Sebrant, Yu.V.; Baranov, V.Yu.; Malyuta, D.D.; Nyz'ev, V.G.

1978-01-01

The sensitivity of yeast cells of different ploidy and bacterial cells of different strains to pulsed laser radiation and combined action of laser and ionizing radiation has been studied. Laser preirradiation of yeast cells did not change the cell sensitivity to the ionizing radiation. The biological effect was non-additive after the exposure to sequence of pulses in comparison with the exposure to a single pulse. The failure of cell reproductive ability after laser irradiation was irrepairable

Efficient femtosecond mid-infrared pulse generation by dispersivewave radiation in bulk lithium niobate crystal

DEFF Research Database (Denmark)

Zhou, Binbin; Guo, Hairun; Bache, Morten

2014-01-01

We experimentally demonstrate efficient mid-infrared pulse generation by dispersive wave radiation in bulk lithium niobate crystal. Femtosecond mid-IR pulses centering from 2.8–2.92 µm are generated using the single pump wavelengths from 1.25–1.45 µm.......We experimentally demonstrate efficient mid-infrared pulse generation by dispersive wave radiation in bulk lithium niobate crystal. Femtosecond mid-IR pulses centering from 2.8–2.92 µm are generated using the single pump wavelengths from 1.25–1.45 µm....

Pure-Phase Selective Excitation in Fast-Relaxing Systems

Science.gov (United States)

Zangger, Klaus; Oberer, Monika; Sterk, Heinz

2001-09-01

Selective pulses have been used frequently for small molecules. However, their application to proteins and other macromolecules has been limited. The long duration of shaped-selective pulses and the short T2 relaxation times in proteins often prohibited the use of highly selective pulses especially on larger biomolecules. A very selective excitation can be obtained within a short time by using the selective excitation sequence presented in this paper. Instead of using a shaped low-intensity radiofrequency pulse, a cluster of hard 90° pulses, delays of free precession, and pulsed field gradients can be used to selectively excite a narrow chemical shift range within a relatively short time. Thereby, off-resonance magnetization, which is allowed to evolve freely during the free precession intervals, is destroyed by the gradient pulses. Off-resonance excitation artifacts can be removed by random variation of the interpulse delays. This leads to an excitation profile with selectivity as well as phase and relaxation behavior superior to that of commonly used shaped-selective pulses. Since the evolution of scalar coupling is inherently suppressed during the double-selective excitation of two different scalar-coupled nuclei, the presented pulse cluster is especially suited for simultaneous highly selective excitation of N-H and C-H fragments. Experimental examples are demonstrated on hen egg white lysozyme (14 kD) and the bacterial antidote ParD (19 kD).

Nonresonant interaction of ultrashort electromagnetic pulses with multilevel quantum systems

Science.gov (United States)

Belenov, E.; Isakov, V.; Nazarkin, A.

1994-01-01

Some features of the excitation of multilevel quantum systems under the action of electromagnetic pulses which are shorter than the inverse frequency of interlevel transitions are considered. It is shown that the interaction is characterized by a specific type of selectivity which is not connected with the resonant absorption of radiation. The simplest three-level model displays the inverse population of upper levels. The effect of an ultrashort laser pulse on a multilevel molecule was regarded as an instant reception of the oscillation velocity by the oscillator and this approach showed an effective excitation and dissociation of the molecule. The estimations testify to the fact that these effects can be observed using modern femtosecond lasers.

Analysis of the Interaction of Pulsed Laser with Nanoporous Activated Carbon Cloth

Institute of Scientific and Technical Information of China (English)

B.V. Kalucljerovic; M.S. Trtica; B.B. Radak; J.M. Stasic; S.S. Krstic Musovic; V.M. Dodevski

2011-01-01

Interaction of pulsed transversely excited atmospheric （TEA） CO2-1aser radiation at 10.6 μm with nanoporous activated carbon cloth was investigated. Activated carbon cloth of different adsorption characteristics was used. Activated carbon cloth modifications were initiated by laser pulse intensities from 0.5 to 28 MW/cm^2, depending on the cloth adsorption characteristics. CO2 laser radiation was effectively absorbed by the used activated carbon cloth and largely converted into thermal energy. The type of modification depended on laser power density, number of pulses, but mostly on material characteristics such as specific surface area. The higher the surface area of activated carbon cloth, the higher the damage threshold.

Radiative transport and collisional transfer of excitation energy in Cs vapors mixed with Ar or He

International Nuclear Information System (INIS)

Vadla, Cedomil; Horvatic, Vlasta; Niemax, Kay

2003-01-01

This paper is a review (with a few original additions) on the radiative transport and collisional transfer of energy in laser-excited cesium vapors in the presence of argon or helium. Narrow-band excitation of lines with Lorentz, Doppler and Voigt profiles is studied in order to calculate effective rates for pumping of spectral lines with profiles comprising inhomogeneous broadening components. The radiative transport of excitation energy is considered, and a new, simple and robust, but accurate theoretical method for quantitative treatment of radiation trapping in relatively optically thin media is presented. Furthermore, comprehensive lists of experimental values for the excitation energy transfer cross-sections related to thermal collisions in Cs-Ar and Cs-He mixtures are given. Within the collected cross-section data sets, specific regularities with respect to the energy defect, as well as the temperature, are discerned. A particular emphasis is put on the radiative and collisional processes important for the optimization of resonance-fluorescence imaging atomic filters based on Cs-noble gas systems

Pulsed laser radiation therapy of skin tumors

Energy Technology Data Exchange (ETDEWEB)

Kozlov, A.P.; Moskalik, K.G.

1980-11-15

Radiation from a neodymium laser was used to treat 846 patients with 687 precancerous lesions or benign tumors of the skin, 516 cutaneous carcinomas, 33 recurrences of cancer, 51 melanomas, and 508 metastatic melanomas in the skin. The patients have been followed for three months to 6.5 years. No relapses have been observed during this period. Metastases to regional lymph nodes were found in five patients with skin melanoma. Pulsed laser radiation may be successfully used in the treatment of precancerous lesions and benign tumors as well as for skin carcinoma and its recurrences, and for skin melanoma. Laser radiation is more effective in the treatment of tumors inaccessible to radiation therapy and better in those cases in which surgery may have a bad cosmetic or even mutilating effect. Laser beams can be employed in conjunction with chemo- or immunotherapy.

Applications of high order harmonic radiation to UVX-solids interaction: high excitation density in electronic relaxation dynamics and surface damaging

International Nuclear Information System (INIS)

De Grazia, M.

2007-12-01

The new sources of radiation in the extreme-UV (X-UV: 10-100 nm), which deliver spatially coherent, ultra-short and intense pulses, allow studying high flux processes and ultra-fast dynamics in various domains. The thesis work presents two applications of the high-order laser harmonics (HH) to solid state physics. In Part I, we describe the optimization of the harmonic for studies of X-UV/solids interaction. In Part II, we investigate effects of high excitation density in the dynamics of electron relaxation in dielectric scintillator crystals - tungstates and fluorides, using time-resolved luminescence spectroscopy. Quenching of luminescence at short time gives evidence of the competition between radiative and non-radiative recombination of self-trapped excitons (STE). The non-radiative channel is identified to mutual interaction of STE at high excitation density. In Part III, we study the X-UV induced damage mechanism in various materials, either conductor (amorphous carbon) or insulators (organic polymers, e.g., PMMA). In PMMA-Plexiglas, in the desorption regime (0.2 mJ/cm 2 , i.e., below damage threshold), the surface modifications reflect X-UV induced photochemical processes that are tentatively identified, as a function of dose: at low dose, polymer chain scission followed by the blow-up of the volatile, low-molecular fragments leads to crater formation; at high dose, cross-linking in the near-surface layer of remaining material leads to surface hardening. These promising results have great perspectives considering the performances already attained and planned in the next future in the development of the harmonic sources. (author)

Interaction of femtosecond X-ray pulses with periodical multilayer structures

International Nuclear Information System (INIS)

Ksenzov, Dmitry

2010-01-01

The VUV Free Electron Laser FLASH operates in soft X-ray range and produces high-intensive pulse trains with few tens femtoseconds duration. The transversely fully coherent beam will open new experiments in solid state physics which can not be studied with present radiation sources. The study of the time dependent response of the multilayer to the X-ray pulse can provide insights into the process of interaction of highly intense FEL radiation with matter. To test the influence of electron excitation on the optical properties of boron carbide, the refractive index of B 4 C was measured near B K-edge by energy-resolved photon-in-photon-out method probing a Bragg reflection from periodical multilayers. The measured data clearly show that the variation of the fine structure of the Kabsorption edges due to the chemical nature of the absorber element. The knowledge obtained from experiments with continuous radiation was used to design the respective experiments with pulse from the FEL. In my thesis, it is proposed that the geometrical setup, where the incident pulse arrives from the FEL under the angle close to the 1st order ML Bragg peak, provides the most valuable information. Preliminary simulation considering form factors of neutral and ionized boron showed that due to ionization, pronounced changes in the reflectivity curve are expected. The proposed scheme can be the powerful tool to study the various processes within the electronic subsystem of the FEL pulse interaction with matter. This type of investigations gives a deep understanding of the nature of the electronic excitation and the recombination at the femtosecond scale. (orig.)

Interaction of femtosecond X-ray pulses with periodical multilayer structures

Energy Technology Data Exchange (ETDEWEB)

Ksenzov, Dmitry

2010-07-01

The VUV Free Electron Laser FLASH operates in soft X-ray range and produces high-intensive pulse trains with few tens femtoseconds duration. The transversely fully coherent beam will open new experiments in solid state physics which can not be studied with present radiation sources. The study of the time dependent response of the multilayer to the X-ray pulse can provide insights into the process of interaction of highly intense FEL radiation with matter. To test the influence of electron excitation on the optical properties of boron carbide, the refractive index of B{sub 4}C was measured near B K-edge by energy-resolved photon-in-photon-out method probing a Bragg reflection from periodical multilayers. The measured data clearly show that the variation of the fine structure of the Kabsorption edges due to the chemical nature of the absorber element. The knowledge obtained from experiments with continuous radiation was used to design the respective experiments with pulse from the FEL. In my thesis, it is proposed that the geometrical setup, where the incident pulse arrives from the FEL under the angle close to the 1st order ML Bragg peak, provides the most valuable information. Preliminary simulation considering form factors of neutral and ionized boron showed that due to ionization, pronounced changes in the reflectivity curve are expected. The proposed scheme can be the powerful tool to study the various processes within the electronic subsystem of the FEL pulse interaction with matter. This type of investigations gives a deep understanding of the nature of the electronic excitation and the recombination at the femtosecond scale. (orig.)

Pulsed radiation studies of carotenoid radicals and excited states

Energy Technology Data Exchange (ETDEWEB)

Burke, M

2001-04-01

The one-electron reduction potentials of the radical cations of five dietary carotenoids, in aqueous micellar environments, have been obtained from a pulse radiolysis study of electron transfer between the carotenoids and tryptophan radical cations as a function of pH, and lie in the range 980 to 1060 mV. The decays of the carotenoid radical cations suggest a distribution of exponential lifetimes. The radicals persist for up to about one second, depending on the medium and may re-orientate within a biological environment to react with other biomolecules, such as tyrosine, cysteine or ascorbic acid, which was indeed confirmed. Spectral information of carotenoid pigmented liposomes has been collected, subsequently pulse radiolysis was used to generate the radical cations of {beta}-carotene, zeaxanthin and lutein, in unilamellar vesicles of dipalmitoyl phosphatidyl choline. The rate constants for the 'repair' of these carotenoid radical cations by water-soluble vitamin C were found to be similar ({approx}1 x 10{sup 7} M{sup -1}s{sup -1}) for {beta}-carotene and zeaxanthin and somewhat lower ({approx}0.5 x 10{sup 7} M{sup -1}s{sup -1}) for lutein. The results are discussed in terms of the microenvironment of the carotenoids and suggest that for {beta}-carotene, a hydrocarbon carotenoid, the radical cation is able to interact with a water-soluble species even though the parent hydrocarbon carotenoid is probably entirely in the non-polar region of the liposome. Studies investigating the ability of ingested lycopene to protect human lymphoid cells against singlet oxygen and nitrogen dioxide radical mediated cell damage have shown that a high lycopene diet is beneficial in protecting human cells against reactive oxygen species. Triplet states of carotenoids were produced in benzene solvent and their triplet lifetimes were found to depend on the concentration of the parent molecule. The rate constants obtained for ground state quenching correlate with the number

Ultrafast molecular dynamics illuminated with synchrotron radiation

International Nuclear Information System (INIS)

Bozek, John D.; Miron, Catalin

2015-01-01

Highlights: • Ultrafast molecular dynamics probed with synchrotron radiation. • Core-excitation as probe of ultrafast dynamics through core-hole lifetime. • Review of experimental and theoretical methods in ultrafast dynamics using core-level excitation. - Abstract: Synchrotron radiation is a powerful tool for studying molecular dynamics in small molecules in spite of the absence of natural matching between the X-ray pulse duration and the time scale of nuclear motion. Promoting core level electrons to unoccupied molecular orbitals simultaneously initiates two ultrafast processes, nuclear dynamics on the potential energy surfaces of the highly excited neutral intermediate state of the molecule on the one hand and an ultrafast electronic decay of the intermediate excited state to a cationic final state, characterized by a core hole lifetime. The similar time scales of these processes enable core excited pump-probe-type experiments to be performed with long duration X-ray pulses from a synchrotron source. Recent results obtained at the PLIEADES beamline concerning ultrafast dissociation of core excited states and molecular potential energy curve mapping facilitated by changes in the geometry of the short-lived intermediate core excited state are reviewed. High brightness X-ray beams combined with state-of-the art electron and ion-electron coincidence spectrometers and highly sophisticated theoretical methods are required to conduct these experiments and to achieve a full understanding of the experimental results.

Calibrated Pulse-Thermography Procedure for Inspecting HDPE

Directory of Open Access Journals (Sweden)

Mohammed A. Omar

2008-01-01

Full Text Available This manuscript discusses the application of a pulse-thermography modality to evaluate the integrity of a high-density polyethylene HDPE joint for delamination, in nonintrusive manner. The inspected HDPE structure is a twin-cup shape, molded through extrusion, and the inspection system comprises a high-intensity, short-duration radiation pulse to excite thermal emission; the text calibrates the experiment settings (pulse duration, and detector sampling rate to accommodate HDPE bulks thermal response. The acquired thermal scans are processed through new contrast computation named “self-referencing”, to investigate the joint tensile strength and further map its adhesion interface in real-time. The proposed system (hardware, software combination performance is assessed through an ultrasound C-scan validation and further benchmarked using a standard pulse phase thermography (PPT routine.

Ultrafast dynamics of laser-pulse excited semiconductors: non-Markovian quantum kinetic equations with nonequilibrium correlations

Directory of Open Access Journals (Sweden)

V.V.Ignatyuk

2004-01-01

Full Text Available Non-Markovian kinetic equations in the second Born approximation are derived for a two-zone semiconductor excited by a short laser pulse. Both collision dynamics and running nonequilibrium correlations are taken into consideration. The energy balance and relaxation of the system to equilibrium are discussed. Results of numerical solution of the kinetic equations for carriers and phonons are presented.

Fluorescence detection of single molecules using pulsed near-field optical excitation and time correlated photon counting

International Nuclear Information System (INIS)

Ambrose, W.P.; Goodwin, P.M.; Martin, J.C.; Keller, R.A.

1994-01-01

Pulsed excitation, time correlated single photon counting and time gated detection are used in near-field optical microscopy to enhance fluorescence images and measure the fluorescence lifetimes of single molecules of Rhodamine 6G on silica surfaces. Time gated detection is used to reject prompt scattered background and to improve the image signal to noise ratio. The excited state lifetime of a single Rhodamine 6G molecule is found to depend on the position of the near-field probe. We attribute the lifetime variations to spontaneous emission rate alterations by the fluorescence reflected from and quenching by the aluminum coated probe

Comparison of laser diode response to pulsed electrical and radiative excitations

International Nuclear Information System (INIS)

Baggio, J.; Rainsant, J.M.; D'hose, C.; Lalande, P.; Musseau, O.; Leray, J.L.

1996-01-01

The authors have studied the electrical and optical response of two laser diodes under transient irradiation. Both diodes exhibit a positive photocurrent, which adds to the bias current, and a decrease of the optical power until extinction when dose rate is increased. Direct carrier generation in the laser cavity is a second order phenomena. The diode overall response is driven by both the substrate photocurrent and the transient conduction of current confinement regions, which decrease the net current density in the cavity and switches-off the laser emission. This behavior is in good agreement with pulsed electrical characterizations and 2D simulations

Emission characteristics of 6.78-MHz radio-frequency glow discharge plasma in a pulsed mode

Science.gov (United States)

Zhang, Xinyue; Wagatsuma, Kazuaki

2017-07-01

This paper investigated Boltzmann plots for both atomic and ionic emission lines of iron in an argon glow discharge plasma driven by 6.78-MHz radio-frequency (RF) voltage in a pulsed operation, in order to discuss how the excitation/ionization process was affected by the pulsation. For this purpose, a pulse frequency as well as a duty ratio of the pulsed RF voltage was selected as the experimenter parameters. A Grimm-style radiation source was employed at a forward RF power of 70 W and at an argon pressures of 670 Pa. The Boltzmann plot for low-lying excited levels of iron atom was on a linear relationship, which was probably attributed to thermal collisions with ultimate electrons in the negative glow region; in this case, the excitation temperature was obtained in a narrow range of 3300-3400 K, which was hardly affected by the duty ratio as well as the pulse frequency of the pulsed RF glow discharge plasma. This observation suggested that the RF plasma could be supported by a self-stabilized negative glow region, where the kinetic energy distribution of the electrons would be changed to a lesser extent. Additional non-thermal excitation processes, such as a Penning-type collision and a charge-transfer collision, led to deviations (overpopulation) of particular energy levels of iron atom or iron ion from the normal Boltzmann distribution. However, their contributions to the overall excitation/ionization were not altered so greatly, when the pulse frequency or the duty ratio was varied in the pulsed RF glow discharge plasma.

Semi-classical description of Rydberg atoms in strong, single-cycle electromagnetic pulses

International Nuclear Information System (INIS)

Jensen, R.V.; Sanders, M.M.

1993-01-01

Recent experimental measurements of the excitation and ionization of Rydberg atoms by single-cycle, electromagnetic pulses have revealed a variety of novel features. Because many quantum states are strongly coupled by the broadband radiation in the short pulse, the traditional methods of quantum mechanics are inadequate to account for the experimental results. We have therefore developed a semi-classical description of the interaction of both hydrogenic and non-hydrogenic atoms with single-cycle pulses of intense, electromagnetic radiation which is based on the strong correspondence theory of Percival and Richards. This theory, which was originally introduced for the description of strong atomic collisions, accounts for some of the surprising features of the experimental measurements and provides new predictions for future experimental studies

Radiative and nonradiative lifetimes in excited states of Ar, Kr and Xe atoms in Ne matrix

International Nuclear Information System (INIS)

Hahn, U.; Schwentner, N.

1979-10-01

Synchrotron radiation with its intense continuum and its excellent time structure has been exploited for time resolved luminescence spectroscopy in the solid state. By selective excitation of n = 1, n' = 1 and n = 2 exciton states of Xe, Kr and Ar atoms in Ne matrix we were able to identify the emitting states involved. Lifetimes within the cascade of radiative and radiationless relaxation between excited states as well as the radiative lifetimes for transitions to the ground state have been derived from the decay curves. Energy positions and radiative lifetimes of the emitting states correspond quite well with those of the free atoms. Radiative and radiationless relaxation processes take place within the manifold of excited states of the guest atoms. The rate constants for radiationless decay confirm an energy gap law. The order of the radiationless processes reaches in some cases extremely high values. Selection rules for spin and angular momentum are essential to understand the observed radiationless transition rates. (orig.)

Electromagnetic soliton production during interaction of relativistically strong laser pulses with plasma

International Nuclear Information System (INIS)

Bulanov, S.V.; Esirkepov, T.Zh.; Kamenets, F.F.; Naumova, N.M.

1995-01-01

The paper presents the results of a numeric modelling of the propagation of ultra short relativistically strong laser pulses in a rarefied plasma by the 'particle in cell'. Primary attention is paid to the process of the formation of electromagnetic solitons which can not be described in the approximation of envelopes. It is found that under certain conditions a significant portion of pulse energy can transform is solitons. The soliton excitation mechanism is related to a decrease of local frequency of electromagnetic radiation due to the generation of wave plasma waves. From one soliton to a stub of solitons can be generated in the wake of a relatively long pulse depending on the parameters of laser pulse in plasma. Particles are effectively accelerated forwards radiation propagation in the electric field of wake plasma waves. 22 refs., 7 figs

Time-resolved UV spectroscopy on ammonia excited by a pulsed CO2 laser

International Nuclear Information System (INIS)

Holbach, H.

1980-07-01

This work investigates the excitation of ammonia by a pulsed CO 2 laser, in particular the processes associated with collisions with argon. It was prompted by two previous observations: the previously reported infrared multiphoton dissociation of NH 3 under nearly collisionless conditions, and the ill understood excitation mechanism of apparently nonresonant low vibrational levels in the presence of Ar. Based on recent spectroscopic data, all vibrational-rotational levels were determined which are simultaneously excited by different CO 2 laser lines. Transitions between the 1 + and 2 - vibrational levels were also taken into account. The linewidth in these calculations was dominated by power broadening, which generates a half width at half maximum of 0.36 cm -1 at the typical power density of 10 MW/cm 2 . In order to reproduce published experimental absorption data, it proved necessary to take account all transitions within a distance of 20 cm -1 from the laser line. This fact implies in most cases the simultaneous population of a large number of vibrational-rotational levels. The population of levels by absorption or by subsequent collisional processes was probed by time-resolved absorption measurement of vibrational bands and their rotational envelope in the near UV. Time resolution (5...10) was sufficient to observe rotational relaxation within individual vibrational levels. Characteristic differences were found for the various excitation lines. (orig.) [de

Appearance property and mechanism of plume produced by pulsed ultraviolet laser ablating copper

International Nuclear Information System (INIS)

Huang Qingju; Li Fuquan; Wang Honghua

2008-01-01

Time-resolved measurements of plume emission spectra by pulsed ultraviolet laser ablating copper in neon were analyzed, and the photographs of plume from laser ablating copper were taken. The experimental results show that plume has different colours in different ranges. At low pressure the centre layer and middle layer colours of plume are mixed colour, and the outer layer colours of plume are yellow and green. At middle pressure the centre layer and middle layer colours of plume are white, and the outer layer colour of plume is pea green. At high pressure the centre layer and middle layer colours of plume are white, and the outer layer colour of plume is faintness green. The plume range is pressed with the rising of ambient gas pressure, and the range colour gets thin with the rising of ambient gas pressure. The plume excitation radiation mechanism in pulsed ultraviolet laser ablating copper was discussed. The primary excitation radiation mechanism in plume is electron collision energy transfer and atom collision energy transfer at low pressure and middle pressure, and it is electrons Bremsstrahlung and recombination excitation radiation of electron and ion at high pressure. The model can be used to explain the experimental result qualitatively. (authors)

Quantum computer based on activated dielectric nanoparticles selectively interacting with short optical pulses

International Nuclear Information System (INIS)

Gadomskii, Oleg N; Kharitonov, Yu Ya

2004-01-01

The operation principle of a quantum computer is proposed based on a system of dielectric nanoparticles activated with two-level atoms - cubits, in which electric dipole transitions are excited by short intense optical pulses. It is proved that the logical operation (logical operator) CNOT (controlled NOT) is performed by means of time-dependent transfer of quantum information over 'long' (of the order of 10 4 nm) distances between spherical nanoparticles owing to the delayed interaction between them in the optical radiation field. It is shown that one-cubit and two-cubit logical operators required for quantum calculations can be realised by selectively exciting dielectric particles with short optical pulses. (quantum calculations)

Photoemission from excited states in rare gas solids by combining synchrotronradiation with a laser

International Nuclear Information System (INIS)

Bernstorff, S.

1984-09-01

A new spectroscopic method has been developed to study excited states in rare gas solids: Excitons and conductionband-states are populated by synchrotron radiation (photon energy hw SR =5 - 30 eV). Subsequently electrons from these bound or conduction band-states are excited above the vacuum level of the solid by a pulsed dye laser (hw L =1.9 - 3.7 eV). This experimental technique was applied to solid Xe, Kr, Ar and Ne. (orig./GSCH)

Terahertz Pulse Generation in Underdense Relativistic Plasmas: From Photoionization-Induced Radiation to Coherent Transition Radiation

Science.gov (United States)

Déchard, J.; Debayle, A.; Davoine, X.; Gremillet, L.; Bergé, L.

2018-04-01

Terahertz to far-infrared emission by two-color, ultrashort optical pulses interacting with underdense helium gases at ultrahigh intensities (>1019 W /cm2 ) is investigated by means of 3D particle-in-cell simulations. The terahertz field is shown to be produced by two mechanisms occurring sequentially, namely, photoionization-induced radiation (PIR) by the two-color pulse, and coherent transition radiation (CTR) by the wakefield-accelerated electrons escaping the plasma. We exhibit laser-plasma parameters for which CTR proves to be the dominant process, providing terahertz bursts with field strength as high as 100 GV /m and energy in excess of 10 mJ. Analytical models are developed for both the PIR and CTR processes, which correctly reproduce the simulation data.

Radiation detectors based by polymer materials

International Nuclear Information System (INIS)

Cherestes, Margareta; Cherestes, Codrut; Constantinescu, Livia

2004-01-01

Scintillation counters make use of the property of certain chemical compounds to emit short light pulses after excitation produced by the passage of charged particles or photons of high energy. These flashes of light are detected by a photomultiplier tube that converts the photons into a voltage pulse. The light emitted from the detector also can be collected, focussed and dispersed by a CCD detector. The study of the evolution of the light emission and of the radiation damage under irradiation is a primary topic in the development of radiation hard polymer based scintillator. Polymer scintillator thin films are used in monitoring radiation beam intensities and simultaneous counting of different radiations. Radiation detectors have characteristics which depend on: the type of radiation, the energy of radiation, and the material of the detector. Three types of polymer thin films were studied: a polyvinyltoluene based scintillator, fluorinated polyimide and PMMA. (authors)

Photocurrent and photovoltage induced in a 2DEG under intense, pulsed THz radiation

International Nuclear Information System (INIS)

Lewis, R.A.; Xu, W.; Pellemans, H.P.M.; Langerak, C.J.G.M.

1999-01-01

Full text: Intense THz radiation emitted by FELIX (Free Electron Laser for Infrared eXperiments) induces both photovoltage and photocurrent signals in a high-mobility (μ = 2 x 10 6 cm 2 /V s), low-density (n e = 2 x 10 11 cm -2 ) GaAs/AlGaAs-based 2DEG. Within the ∼5 μs FELIX macropulse, there is a rapid response in the longitudinal voltage of a Hall-bar sample, reproducible between pulses. A large response continues well after the pulse; this long-time-scale behaviour varies between pulses if the current exceeds a critical value (which decreases with radiation intensity and magnetic field). Within the macropulse, the photovoltage varies with magnetic field, saturating at low field (<100 mT). The photocurrent shows a rapid, non-resonant response, evident at integral filling factors in both longitudinal and transverse data, and a slower, cyclotron resonant response, peaking at ∼390 μs after the FELIX pulse. No anisotropy in the resistivity under polarised radiation was found

Dc to ac field conversion due to leaky-wave excitation in a plasma slab behind an ionization front

International Nuclear Information System (INIS)

Kostin, V A; Vvedenskii, N V

2015-01-01

We present a way for generating coherent tunable electromagnetic radiation through dc to ac field conversion by an ionization front. The conversion is caused by the excitation of leaky waves behind the transversely limited ionization front propagating in a uniform electrostatic field. This differs significantly from the well-known dc-to-ac-radiation-converter models which consider Doppler-like frequency conversion by a transversely unlimited ionization front propagating in a spatially periodic electric field. We explore the dispersion properties and excitation of these leaky waves radiated through the transverse plasma boundary at the Cherenkov angle to the direction of propagation of a superluminal ionization front as dependent on the parameters of the plasma produced and on the speed of the ionization front. It is shown that not only the center frequency but also the duration and waveform of the generated pulse may significantly depend on the speed of the ionization front. The results indicate the possibility of using such converters based on planar photoconductive antennas to create sources of microwave and terahertz radiation with controllable waveforms that are transformed from video to radio pulse when the angle of incident ionizing radiation is tuned. (paper)

The triplet excited state of bilirubin

International Nuclear Information System (INIS)

Land, E.J.

1976-01-01

Pulse radiolysis of benzene solutions of 40 μM bilirubin alone or with 0.1 M biphenyl has yielded evidence for the formation of the triplet excited state of bilirubin. Measurements were made of a number of properties, including the absorption spectrum (lambdasub(max)500nm), lifetime 9μs), extinction coefficient (8800 M -1 cm -1 ), energy level (approximately 150 kJ mol -1 ) and the rate of quenching by oxygen (rate constant, 8.2 x 10 8 M -1 s -1 ). An upper limit of 0.1 has also been obtained for the singlet to triplet crossover efficiency of bilirubin following excitation by 353 nm radiation. Consideration is given to the relevance of these data to the mechanism of bilirubin photo-destruction, both in vivo and in vitro. (U.K.)

Emission Behavior of Crystalline 1,4-Bis(4-phenylthiophene-2-yl)benzene Film Under Optical Excitation with Ultra Short Pulses.

Science.gov (United States)

Mochizuki, Hiroyuki; Kawaguchi, Yoshizo; Sasaki, Fumio; Hotta, Shu

2016-04-01

We evaluated emission behaviors of crystallized films of 1,4-bis(5-phenylthiophene-2-yl)benzene (AC5) in detail which was a representative thiophene/phenylene co-oligomer. The crystallized AC5 films were prepared by vapor deposition onto a substrate and thermal treatment. The AC5 films consisted of a crystalline domain with the size of several tens of micrometers. We used femtosecond laser pulses for the excitation of the AC5 films. As a result, the femtosecond laser pulses did not induce re-absorption above excitation energy densities of their laser threshold. The obtained gain value for AC5 crystallized film was large, over 150 cm-1. Furthermore, the emission cross section of the crystallized AC5 film was nearly 10(-16) cm2.

Investigation of collisional excitation-transfer processes in a plasma by laser perturbation method

International Nuclear Information System (INIS)

Sakurai, Takeki

1983-01-01

The theoretical background and the experimental method of the laser perturbation method applied to the study of collisional excitation transfer process in plasma are explained. The atomic density at some specified level can be evaluated theoretically. By using the theoretical results and the experimentally obtained data, the total attenuation probability, the collisional transfer probability and natural emission probability were estimated. For the experiments, continuous wave laser (cw) and pulse laser are employed. It is possible by using pulse dye laser to observe the attenuation curve directly, and to bring in resonance to any atomic spectra. At the beginning, the experimental studies were made on He-Ne discharge. The pulse dye laser has been used for the excitation of alkali atoms. The first application of pulse laser to the study of plasma physics was the study on He. The cross section of disalignment has also been studied by the laser perturbation. The alignment of atoms, step and cascade transfer, the confinement of radiation and optogalvanic effect are discussed in this paper. (Kato, T.)

Experimental study of the counting loss in an ionization chamber in pulsed radiation fields

International Nuclear Information System (INIS)

Goncalez, O.L.; Yanagihara, L.S.; Veissid, V.L.C.P.; Herdade, S.B.; Teixeira, A.N.

1983-01-01

The behavior of an ionization chamber gamma ray monitor in a pulsed radiation field at a linear electron accelerator facility was studied experiementally. A loss of sensitivity was observed as expected due to the pulsed nature of the radiation. By fitting the experiemental data to semi-empirical expressions, parameters for the correction of the counting efficiency were obtained. (Author) [pt

Excitation of low-frequency residual currents at combination frequencies of an ionising two-colour laser pulse

Science.gov (United States)

Vvedenskii, N. V.; Kostin, V. A.; Laryushin, I. D.; Silaev, A. A.

2016-05-01

We have studied the processes of excitation of low-frequency residual currents in a plasma produced through ionisation of gases by two-colour laser pulses in laser-plasma schemes for THz generation. We have developed an analytical approach that allows one to find residual currents in the case when one of the components of a two-colour pulse is weak enough. The derived analytical expressions show that the effective generation of the residual current (and hence the effective THz generation) is possible if the ratio of the frequencies in the two-colour laser pulse is close to a rational fraction with a not very big odd sum of the numerator and denominator. The results of numerical calculations (including those based on the solution of the three-dimensional time-dependent Schrödinger equation) agree well with the analytical results.

Scattering of an ultrashort electromagnetic radiation pulse by an atom in a broad spectral range

International Nuclear Information System (INIS)

Astapenko, V. A.

2011-01-01

The scattering of an ultrashort electromagnetic pulse by atomic particles is described using a consistent quantum-mechanical approach taking into account excitation of a target and nondipole electromagnetic interaction, which is valid in a broad spectral range. This approach is applied to the scattering of single- and few-cycle pulses by a multielectron atom and a hydrogen atom. Scattering spectra are obtained for ultrashort pulses of different durations. The relative contribution of “elastic” scattering of a single-cycle pulse by a hydrogen atom is studied in the high-frequency limit as a function of the carrier frequency and scattering angle.

Microwave radiation mechanism in a pulse-laser-irradiated Cu foil target revisited

International Nuclear Information System (INIS)

Chen Ziyu; Li Jianfeng; Li Jun; Peng Qixian

2011-01-01

The microwave radiation mechanism in a Cu-based foil target irradiated by an intense laser pulse has been investigated. Microwave emission in the frequency range 0.5-4 GHz has been observed from a 200 ps laser pulse of intensity about 10 12 W cm -2 normally incident on the target surface. The total microwave power and energy emitted from the interaction were found to be about 0.4 W and 2 nJ, respectively, corresponding to an efficiency of coupling laser energy to microwave energy of 2x10 -8 . The result agrees well with quadrupole radiation calculated based on a circuit model of a laser plasma, which indicates that the radiative process can be explained by magnetic dipole or electric quadrupole radiation from the laser-produced symmetric poloidal current distribution at the plasma-target interface.

Microwave radiation mechanism in a pulse-laser-irradiated Cu foil target revisited

Energy Technology Data Exchange (ETDEWEB)

Chen Ziyu; Li Jianfeng; Li Jun; Peng Qixian, E-mail: ziyuch@gmail.com [Institute of Fluid Physics, China Academy of Engineering Physics, Mianyang 621900 (China)

2011-05-01

The microwave radiation mechanism in a Cu-based foil target irradiated by an intense laser pulse has been investigated. Microwave emission in the frequency range 0.5-4 GHz has been observed from a 200 ps laser pulse of intensity about 10{sup 12} W cm{sup -2} normally incident on the target surface. The total microwave power and energy emitted from the interaction were found to be about 0.4 W and 2 nJ, respectively, corresponding to an efficiency of coupling laser energy to microwave energy of 2x10{sup -8}. The result agrees well with quadrupole radiation calculated based on a circuit model of a laser plasma, which indicates that the radiative process can be explained by magnetic dipole or electric quadrupole radiation from the laser-produced symmetric poloidal current distribution at the plasma-target interface.

Thermomechanical effect of pulse-periodic laser radiation on cartilaginous and eye tissues

Science.gov (United States)

Baum, O. I.; Zheltov, G. I.; Omelchenko, A. I.; Romanov, G. S.; Romanov, O. G.; Sobol, E. N.

2013-08-01

This paper is devoted to theoretical and experimental studies into the thermomechanical action of laser radiation on biological tissues. The thermal stresses and strains developing in biological tissues under the effect of pulse-periodic laser radiation are theoretically modeled for a wide range of laser pulse durations. The models constructed allow one to calculate the magnitude of pressures developing in cartilaginous and eye tissues exposed to laser radiation and predict the evolution of cavitation phenomena occurring therein. The calculation results agree well with experimental data on the growth of pressure and deformations, as well as the dynamics of formation of gas bubbles, in the laser-affected tissues. Experiments on the effect of laser radiation on the trabecular region of the eye in minipigs demonstrated that there existed optimal laser irradiation regimens causing a substantial increase in the hydraulic permeability of the radiation-exposed tissue, which can be used to develop a novel glaucoma treatment method.

Thermomechanical effect of pulse-periodic laser radiation on cartilaginous and eye tissues

International Nuclear Information System (INIS)

Baum, O I; Omelchenko, A I; Sobol, E N; Zheltov, G I; Romanov, G S; Romanov, O G

2013-01-01

This paper is devoted to theoretical and experimental studies into the thermomechanical action of laser radiation on biological tissues. The thermal stresses and strains developing in biological tissues under the effect of pulse-periodic laser radiation are theoretically modeled for a wide range of laser pulse durations. The models constructed allow one to calculate the magnitude of pressures developing in cartilaginous and eye tissues exposed to laser radiation and predict the evolution of cavitation phenomena occurring therein. The calculation results agree well with experimental data on the growth of pressure and deformations, as well as the dynamics of formation of gas bubbles, in the laser-affected tissues. Experiments on the effect of laser radiation on the trabecular region of the eye in minipigs demonstrated that there existed optimal laser irradiation regimens causing a substantial increase in the hydraulic permeability of the radiation-exposed tissue, which can be used to develop a novel glaucoma treatment method. (paper)

Silicon dioxide etching process for fabrication of micro-optics employing pulse-modulated electron-beam-excited plasma

International Nuclear Information System (INIS)

Takeda, Keigo; Ohta, Takayuki; Ito, Masafumi; Hori, Masaru

2006-01-01

Silicon dioxide etching process employing a pulse-modulated electron-beam-excited plasma (EBEP) has been developed for a fabrication process of optical micro-electro-mechanical systems (MEMSs). Nonplanar dielectric materials were etched by using self-bias induced by the electron beam generating the plasma. In order to investigate the effect of pulse modulation on electron beam, plasma diagnostics were carried out in the EBEP employing C 4 F 8 gas diluted with Ar gas by using a Langmuir single probe and time resolved optical emission spectroscopy. It was found that the pulse-modulated EBEP has an excellent potential to reduce the plasma-induced thermal damage on a photoresist film on a substrate to get the uniform etching and the anisotropic SiO 2 etching in comparison with the conventional EBEP. The pulse-modulated EBEP enabled us to get the high etch rate of SiO 2 of 375 nm/min without any additional bias power supply. Furthermore, the microfabrication on the core area of optical fiber was realized. These results indicate that the pulse-modulated EBEP will be a powerful tool for the application to optical MEMS process

Dynamic modification of the fragmentation of COq+ excited states generated with high-order harmonics

International Nuclear Information System (INIS)

Cao, W.; De, S.; Singh, K. P.; Chen, S.; Laurent, G.; Ray, D.; Ben-Itzhak, I.; Cocke, C. L.; Schoeffler, M. S.; Belkacem, A.; Osipov, T.; Rescigno, T.; Alnaser, A. S.; Bocharova, I. A.; Zherebtsov, S.; Kling, M. F.; Litvinyuk, I. V.

2010-01-01

The dynamic process of fragmentation of CO q+ excited states is investigated using a pump-probe approach. EUV radiation (32-48 eV) generated by high-order harmonics was used to ionize and excite CO molecules and a time-delayed infrared (IR) pulse (800 nm) was used to influence the evolution of the dissociating multichannel wave packet. Two groups of states, separable experimentally by their kinetic-energy release (KER), are populated by the EUV and lead to C + -O + fragmentation: direct double ionization of the neutral molecule and fragmentation of the cation leading to C + -O*, followed by autoionization of O*. The IR pulse was found to modify the KER of the latter group in a delay-dependent way which is explained with a model calculation.

Decay, excitation, and ionization of lithium Rydberg states by blackbody radiation

Science.gov (United States)

Ovsiannikov, V. D.; Glukhov, I. L.

2010-09-01

Details of interaction between the blackbody radiation and neutral lithium atoms were studied in the temperature ranges T = 100-2000 K. The rates of thermally induced decays, excitations and ionization were calculated for S-, P- and D-series of Rydberg states in the Fues' model potential approach. The quantitative regularities for the states of the maximal rates of blackbody-radiation-induced processes were determined. Approximation formulas were proposed for analytical representation of the depopulation rates.

Excitation and ionization of hydrogen and helium atoms by femtosecond laser pulses: theoretical approach by Coulomb-Volkov states

International Nuclear Information System (INIS)

Guichard, R.

2007-12-01

We present a theoretical approach using Coulomb-Volkov states that appears useful for the study of atomic multi-photonic processes induced by intense XUV femtosecond laser pulses. It predicts hydrogen ionization spectra when it is irradiated by laser pulses in perturbations conditions. Three ways have been investigated. Extension to strong fields when ℎω > I p : it requires to include the hydrogen ground state population, introducing it in standard Coulomb-Volkov amplitude leads to saturated multi-photonic ionization. Extension to multi-photonic transitions with ℎω p : new quantum paths are open by the possibility to excite the lower hydrogen bound states. Multiphoton excitation of these states is investigated using a Coulomb-Volkov approach. Extension to helium: two-photon double ionization study shows the influence of electronic correlations in both ground and final state. Huge quantity of information such as angular and energetic distributions as well as total cross sections is available. (author)

Inner-shell excitation and site specific fragmentation of poly(methylmethacrylate) thin film

Science.gov (United States)

Tinone, Marcia C. K.; Tanaka, Kenichiro; Maruyama, Junya; Ueno, Nobuo; Imamura, Motoyasu; Matsubayashi, Nobuyuki

1994-04-01

Soft x-ray excitations in the 250-600 eV photon energy range on poly(methylmethacrylate) (PMMA) result in ionic fragmentation of the original polymer with the most intense ions corresponding to CH+3, H+, CH+2, CH+, CHO+, and COOCH+3. The photon energy dependence of ion desorption from thin films of PMMA was measured to investigate the primary steps in radiation induced decomposition following carbon and oxygen 1s electron excitations using monochromatic pulsed-synchrotron radiation. It was clearly found that the decomposition depends on the nature of the electronic states created in the excited species. The fragmentation pattern changes depending on the transitions of the 1s electron to a Rydberg orbital, an unoccupied molecular orbital or the ionization continuum. Moreover, the fragmentation occurs specifically around the site of the atom where the optical excitation takes place. Excitations from carbon and oxygen 1s to σ* states seem to be specially efficient for ion production as observed in the case of CH+3, CH+2, and CH+ at 288.7 and 535.6 eV, and in the case of CHO+ at 539.3 eV.

Powerful highly efficient KrF lamps excited by surface and barrier discharges

International Nuclear Information System (INIS)

Borisov, V M; Vodchits, V A; El'tsov, A V; Khristoforov, O B

1998-01-01

An investigation was made of the characteristics of KrF lamps with different types of excitation by surface and barrier discharges in which the dielectric material was sapphire. The conditions were determined for the attainment of an extremely high yield of the KrF* fluorescence with the internal efficiency η in ∼30 % and 22% for pulsed surface and barrier discharges, respectively. A homogeneous surface discharge was maintained without gas circulation when the pulse repetition rate was 5 x 10 4 Hz. Quasicontinuous excitation of a surface discharge at near-atmospheric pressure made it possible to reach a KrF* fluorescence power density of about 80 W cm -3 , which was close to the limit set by the kinetics of the gaseous medium. Under prolonged excitation conditions the intensity of the UV output radiation was limited by the permissible heating of the gas to a temperature above which the operating life of the gaseous mixture containing fluorine fell steeply. This was the reason for the advantage of surface over barrier discharges: the former were characterised by a high thermal conductivity of a thin (∼0.2 mm) plasma layer on the surface of the cooled dielectric, which made it possible to construct powerful highly efficient KrF and ArF lamps emitting UV radiation of up to 1 W cm -2 intensity. (laser system components)

Pulsed neutron well logging apparatus having means for determining background radiation

International Nuclear Information System (INIS)

Randall, R.R.

1979-01-01

A neutron generator in a well logging instrument is periodically pulsed and has an off period between pulses of 1000 microseconds. A neutron detector is gated on at intervals of 400 to 500, 550 to 650, and 700 to 800 microseconds, respectively, following the termination of each burst of fast neutrons. Circuitry is provided for determining the background radiation and for determining the macroscopic absorption. 3 claims

Pulsed electron accelerator for radiation technologies in the enviromental applications

Science.gov (United States)

Korenev, Sergey

1997-05-01

The project of pulsed electron accelerator for radiation technologies in the environmental applications is considered. An accelerator consists of high voltage generator with vacuum insulation and vacuum diode with plasma cathode on the basis discharge on the surface of dielectric of large dimensions. The main parameters of electron accelerators are following: kinetic energy 0.2 - 2.0 MeV, electron beam current 1 - 30 kA and pulse duration 1- 5 microseconds. The main applications of accelerator for decomposition of wastewaters are considered.

Activation of neuron generator of luciola mingrelica luminescence flashes under the effect of pulse X-radiation

International Nuclear Information System (INIS)

Bol'shakov, V.Yu.; Drobchenko, E.A.; Landa, S.B.; Pejmer, S.I.

1990-01-01

The effect of low-level pulse X-radiation on spontaneous photoactivity and luminous communicative behaviour of Luciola mingrelica has been investigated. It was shown that X-radiation doses of as low as 5x10 -5 Gy increased endogenous flashing activity and disinhibited the reaction of insects to light flashes imitating signals of mating partners. Powerful radiation pulses may influence significantly an instinctive behaviour and its neuronal organization

Radiation-induced conductivity of doped silicon in response to photon, proton and neutron irradiation

International Nuclear Information System (INIS)

Kishimoto, N.; Amekura, H.; Plaksin, O.A.; Stepanov, V.A.

2000-01-01

The opto-electronic performance of semiconductors during reactor operation is restricted by radiation-induced conductivity (RIC) and the synergistic effects of neutrons/ions and photons. The RICs of Si due to photons, protons and pulsed neutrons have been evaluated, aiming at radiation correlation. Protons of 17 MeV with an ionizing dose rate of 10 3 Gy/s and/or photons (hν=1.3 eV) were used to irradiate impurity-doped Si (2x10 16 B atoms/cm 3 ) at 300 and 200 K. Proton-induced RIC (p-RIC) and photoconductivity (PC) were intermittently detected in an accelerator device. Neutron-induced RIC (n-RIC) was measured for the same Si in a pulsed fast-fission reactor, BARS-6, with a 70-μs pulse of 2x10 12 n/cm 2 (E>0.01 MeV) and a dose rate of up to 6x10 5 Gy/s. The neutron irradiation showed a saturation tendency in the flux dependence at 300 K due to the strong electronic excitation. Normalization of the electronic excitation, including the pulsed regime, gave a fair agreement among the different radiation environments. Detailed comparison among PC, p-RIC and n-RIC is discussed in terms of radiation correlation including the in-pile condition

Area radiation monitor at the intense pulsed-neutron source

International Nuclear Information System (INIS)

Eichholz, J.J.; Lynch, F.J.; Mundis, R.L.; Howe, M.L.; Dolecek, E.H.

1981-01-01

A tissue-equivalent ionization chamber with associated circuitry has been developed for area radiation monitoring in the Intense Pulsed-Neutron Source (IPNS) facility at Argonne National Laboratory. The conventional chamber configuration was modified in order to increase the electric field and effective volume thereby achieving higher sensitivity and linearity. The instrument provides local and remote radiation level indications and a high level alarm. Twenty-four of these instruments were fabricated for use at various locations in the experimental area of the IPNS-1 facility

Properties of spectra of the reflected and transmitted radiation during propagation of relativistically strong laser pulses in underdense plasmas

International Nuclear Information System (INIS)

Bulanov, S.V.; Esirkepov, T.Z.; Naumova, N.M.

1996-01-01

Particle-in-cell simulation has been performed to study the spatial-temporal evolution of the pulse propagating in an underdense plasma. The spectra both of the reflected and transmitted radiation are investigated. The spectrum structure of the reflected radiation is due to the backward stimulated Raman scattering meanwhile the transmitted radiation structure is mainly due to the nonlinear self-phase-modulation. The influence of the pulse shape on the transmitted radiation spectrum is revealed. The dependence of the main features of the spectrum and the self-consistent pulse distortion is found. The pulse distortion is accompanied by the relativistic electrons generation. copyright 1996 American Institute of Physics

Pulsed electromagnetic field radiation from a narrow slot antenna with a dielectric layer

NARCIS (Netherlands)

Štumpf, M.; De Hoop, A.T.; Lager, I.E.

2010-01-01

Analytic time domain expressions are derived for the pulsed electromagnetic field radiated by a narrow slot antenna with a dielectric layer in a two?dimensional model configuration. In any finite time window of observation, exact pulse shapes for the propagated, reflected, and refracted wave

Effect of gamma radiation on egg hatchability of bruchids developing in three pulses

International Nuclear Information System (INIS)

Nagrare, V.S.; Bhatia, Parvathy

2000-01-01

One day old adults of Callosobruchus chinensis (Linn.) and Callosobruchus maculatus (Fab.) irradiated at 5, 10, 15, 20, 25, 30, 35 Gy dose of gamma radiation were bred on three pulses. Percent egg hatchability was inversely related with gamma radiation dose in both the species on three pulses and it was comparatively low in C. maculatus (Fab.). The mean percent hatchability was 70.66, 68.94, 65.41 on green gram, chickpea and cowpea, respectively in C. chinensis (Linn.) while in C. maculatus (Fab.) it was 66.52, 64.12, 61.27 on green gram, cowpea, chickpea, respectively. Both bruchids tolerated in the radiation doses when bred on green gram whereas they were susceptible on cowpea and chickpea. (author)

[Atomic/ionic fluorescence in microwave plasma torch discharge with excitation of high current and microsecond pulsed hollow cathode lamp: Ca atomic/ionic fluorescence spectrometry].

Science.gov (United States)

Gong, Zhen-bin; Liang, Feng; Yang, Peng-yuan; Jin, Qin-han; Huang, Ben-li

2002-02-01

A system of atomic and ionic fluorescence spectrometry in microwave plasma torch (MPT) discharge excited by high current microsecond pulsed hollow cathode lamp (HCMP HCL) has been developed. The operation conditions for Ca atomic and ionic fluorescence spectrometry have been optimized. Compared with atomic fluorescence spectrometry (AFS) in argon microwave induced plasma (MIP) and MPT with the excitation of direct current and conventional pulsed HCL, the system with HCMP HCL excitation can improve AFS and ionic fluorescence spectrometry (IFS) detection limits in MPT atomizer and ionizer. Detection limits (3 sigma) with HCMP HCL-MPT-AFS/IFS are 10.1 ng.mL-1 for Ca I 422.7 nm, 14.6 ng.mL-1 for Ca II 393.4 nm, and 37.4 ng.mL-1 for Ca II 396.8 nm, respectively.

Quadri-Pulse Theta Burst Stimulation using Ultra-High Frequency Bursts - A New Protocol to Induce Changes in Cortico-Spinal Excitability in Human Motor Cortex

DEFF Research Database (Denmark)

Jung, Nikolai H; Gleich, Bernhard; Gattinger, Norbert

2016-01-01

Patterned transcranial magnetic stimulation (TMS) such as theta burst stimulation (TBS) or quadri-pulse stimulation (QPS) can induce changes in cortico-spinal excitability, commonly referred to as long-term potentiation (LTP)-like and long-term depression (LTD)-like effects in human motor cortex (M...... of sinusoidal TMS pulses elicited either a posterior-anterior (PA) or anterior-posterior (AP) directed current in M1. Motor evoked potentials (MEPs) were recorded before and after qTBS to probe changes in cortico-spinal excitability. PA-qTBS at 666 Hz caused a decrease in PA-MEP amplitudes, whereas AP...... in cortico-spinal excitability. Induced current direction in the brain appears to be relevant when qTBS targets I-wave periodicity, corroborating that high-fidelity spike timing mechanisms are critical for inducing bi-directional plasticity in human M1....

Radiation-driven hydrodynamics of long pulse hohlraums on the National Ignition Facility

International Nuclear Information System (INIS)

Dewald, D L; Landen, O L; Suter, L J; Schein, J; Holder, J.; Campbell, K.; Glenzer, S H.; McDonald, J W.; Niemann, C.; Mackinnon, A J.; Schneider, M S.; Haynam, C.; Hinkel, D.; Hammel, B.A.

2005-01-01

The first hohlraum experiments on the National Ignition Facility (NIF) using the first four laser beams have activated the indirect drive experimental capabilities and tested radiation temperature limits imposed by hohlraum plasma filling. Vacuum hohlraums have been irradiated with laser powers up to 6 TW, 1 ns to 9 ns long square pulses and energies of up to 17 kJ to activate several diagnostics, to study the hohlraum radiation temperature scaling with the laser power and hohlraum size, and to make contact with hohlraum experiments performed at the NOVA and Omega laser facilities. Furthermore, for a variety of hohlraum sizes and pulse lengths, the measured x-ray flux shows signatures of plasma filling that coincide with hard x-ray emission from plasma streaming out of the hohlraum. These observations agree with hydrodynamic simulations and with analytical modeling that includes hydrodynamic and coronal radiative losses. The modeling predicts radiation temperature limits on full NIF (1.8 MJ) that are significantly greater than required for ignition hohlraums

Radiation chemistry and advanced polymer materials studied by picosecond pulse radiolysis combined with femtosecond laser

International Nuclear Information System (INIS)

Tagawa, S.; Yoshida, Y.; Miki, M.; Yamamoto, T.; Ushida, K.; Izumi, Y.

1996-01-01

We have synchronized a single picosecond MeV electron pulse from L-band linear accelerator (linac) of The Institute of Scientific and Industrial Research of Osaka University to a single femtosecond laser pulse of Ti:Sapphire laser. It is an essential technique for the future femtosecond pulse radiolysis and is also applied to many kinds of combined application of more than two different beams from accelerators in very short time range. Radiation chemistry and new type of polymers have been studied by LL (laser-linac) twin picosecond pulse radiolysis. Especially the early events in radiation chemistry such as geminate recombination processes of electrons and radical cations are have been studied in both liquids and solids. (author)

Excited-State Dynamics of Melamine and Its Lysine Derivative Investigated by Femtosecond Transient Absorption Spectroscopy

Directory of Open Access Journals (Sweden)

Yuyuan Zhang

2016-11-01

Full Text Available Melamine may have been an important prebiotic information carrier, but its excited-state dynamics, which determine its stability under UV radiation, have never been characterized. The ability of melamine to withstand the strong UV radiation present on the surface of the early Earth is likely to have affected its abundance in the primordial soup. Here, we studied the excited-state dynamics of melamine (a proto-nucleobase and its lysine derivative (a proto-nucleoside using the transient absorption technique with a UV pump, and UV and infrared probe pulses. For melamine, the excited-state population decays by internal conversion with a lifetime of 13 ps without coupling significantly to any photochemical channels. The excited-state lifetime of the lysine derivative is slightly longer (18 ps, but the dominant deactivation pathway is otherwise the same as for melamine. In both cases, the vast majority of excited molecules return to the electronic ground state on the aforementioned time scales, but a minor population is trapped in a long-lived triplet state.

Interference between radiative emission and autoionization in the decay of excited states of atoms

International Nuclear Information System (INIS)

Armstrong, L. Jr.; Theodosiou, C.E.; Wall, M.J.

1978-01-01

An excited state of an atom which can autoionize can also undergo radiative decay. We consider the interaction between the final states resulting from these two modes of decay, and its effects on such quantities as the fluorescence yield of the excited state, excitation profile of the excited state, and the spectra of the emitted photons and electrons. It is shown that the fraction of decays of the excited state resulting in a photon (fluorescence yield) is particularly sensitive to the details of the final-state interaction. In lowest order in the final-state interaction, the fluorescence yield is increased by a factor (1 + 1/q 2 ) from the traditional value, where q is the Fano q parameter relating to the excited state and the final atomic state

Pulsed magnetization transfer contrast MRI by a sequence with water selective excitation

Energy Technology Data Exchange (ETDEWEB)

Schick, F. [Univ. of Tuebingen (Germany)

1996-01-01

A water selective SE imaging sequence was developed providing suitable properties for the assessment of magnetization transfer (MT) effects in tissues with considerable amounts of fat. The sequence with water selective excitation and slice selective refocusing combines the following features: The RIF exposure on the macromolecular protons is relatively low for single slice imaging without MT prepulses, since no additional pulses for fat saturation are necessary. Water selection by frequency selective excitation diminishes faults in the subtraction of images recorded with and without MT prepulses (which might arise from movements). High differences in the signal amplitudes from hyaline cartilage and muscle tissue were obtained comparing images recorded with irradiation of the series of prepulses for MT and those lacking MT prepulses. Utilizations of the described water selective approach for the assessment of MT effects in lesions of cartilage and bone are demonstrated. MT saturation was also examined in muscles with fatty degeneration of patients suffering from progressive muscular dystrophy. The described technique allows determination of MT effects with good precision in a single slice, especially in regions with dominating fat signals. 22 refs., 5 figs.

Widely tunable narrow-band coherent Terahertz radiation from an undulator at THU

Science.gov (United States)

Su, X.; Wang, D.; Tian, Q.; Liang, Y.; Niu, L.; Yan, L.; Du, Y.; Huang, W.; Tang, C.

2018-01-01

There is anxious demand for intense widely tunable narrow-band Terahertz (THz) radiation in scientific research, which is regarded as a powerful tool for the coherent control of matter. We report the generation of widely tunable THz radiation from a planar permanent magnet undulator at Tsinghua University (THU). A relativistic electron beam is compressed by a magnetic chicane into sub-ps bunch length to excite THz radiation in the undulator coherently. The THz frequency can be tuned from 0.4 THz to 10 THz continuously with narrow-band spectrums when the undulator gap ranges from 23 mm to 75 mm. The measured pulse THz radiation energy from 220 pC bunch is 3.5 μJ at 1 THz and tens of μJ pulse energy (corresponding peak power of 10 MW) can be obtained when excited by 1 nC beam extrapolated from the property of coherent radiation. The experimental results agree well with theoretical predictions, which demonstrates a suitable THz source for the many applications that require intense and widely tunable THz sources.

Studies on the optogalvanic effect and isotope-selective excitation of ytterbium in a hollow cathode discharge lamp using a pulsed dye laser.

Science.gov (United States)

Kumar, Pankaj; Kumar, Jitendra; Prakash, Om; Saini, Vinod K; Dixit, Sudhir K; Nakhe, Shankar V

2013-09-01

This paper presents studies on the pulsed optogalvanic effect and isotope-selective excitation of Yb 555.648 nm (0 cm(-1) → 17 992.007 cm(-1)) and 581.067 nm (17 992.007 cm(-1) → 35 196.98 cm(-1)) transitions, in a Yb/Ne hollow cathode lamp. The Yb atoms were excited by narrow linewidth (500-1000 MHz) Rh110 and Rh6G dye based pulsed lasers. Optogalvanic signal inversion for ground state transition at 555.648 nm was observed beyond a hollow cathode discharge current of 8.5 mA, in contrast to normal optogalvanic signal at 581.067 nm up to maximum current of 14 mA. The isotope-selective excitation studies of Yb were carried out by recording Doppler limited optogalvanic signals as a function of dye laser wavelength. For the 581.067 nm transition, three even isotopes, (172)Yb, (174)Yb, and (176)Yb, and one odd isotope, (171)Yb, were clearly resolved. These data were compared with selective isotope excitation by 10 MHz linewidth continuous-wave dye laser. For 555.648 nm transition, isotopes were not clearly resolved, although isotope peaks of low modulation were observed.

Enhanced performance of an EUV light source (λ = 84 nm) using short-pulse excitation of a windowless dielectric barrier discharge in neon

International Nuclear Information System (INIS)

Carman, R J; Kane, D M; Ward, B K

2010-01-01

The electrical and optical characteristics of a dielectric barrier discharge (DBD) based neon excimer lamp generating output in the extreme ultraviolet (EUV) spectral range (λ = 84 nm) have been investigated experimentally. We report a detailed comparison of lamp performance for both pulsed and sinusoidal voltage excitation waveforms, using otherwise identical operating conditions. The results show that pulsed voltage excitation yields a ∼50% increase in the overall electrical to EUV conversion efficiency compared with sinusoidal waveforms, when operating in the pressure range 500-900 mbar. Pulsed operation allows greater control of parameters associated with the temporal evolution of the EUV pulse shapes (risetime, instantaneous peak power). The Ne DBD based source is also found to be highly monochromatic with respect to its spectral output from the second continuum band at λ ∼ 84 nm (5 nm FWHM). This continuum band dominates the spectral emission over the wavelength range 30-550 nm. Lamp performance; as measured by the overall EUV output energy, electrical to EUV conversion efficiency and spectral purity at λ ∼ 84 nm; improves with increasing gas pressure up to p = 900 mbar.

EVALUATION OF THE THERAPEUTIC EFFICACY OF HIGH-INTENSITY PULSED-PERIODIC LASER RADIATION (CLINICAL AND EXPERIMENTAL OBSERVATIONS

Directory of Open Access Journals (Sweden)

V. V. Sokolov

2016-01-01

Full Text Available From the experience of clinical observations, we have shown a high therapeutic effectiveness of the medical laser KULON-MED in: cosmetics, non-cancer inflammatory diseases of the gastrointestinal tract and cancer (cancer of the stomach and colon as at different wavelengths, and with different types of photosensitizers. In the area of anti-tumor photodynamic therapy (PDT, based on experimental studies, we have showed the high antitumor (sarcoma S‑37 effectiveness of the laser (with the inhibition of tumor growth of up to 100% for repetitively pulsed irradiation mode, and for mode fractionation doses laser radiation. In addition, significant differences are shown in the effectiveness of anticancer PDT methods in the application of high-intensity lasers, continuous and pulsed caused fundamental properties of laser radiation characteristics – time structure of the radiation pulses. Thus, for the first time we have shown that the time of high-intensity laser pulses structure significantly affects therapeutic efficacy laser system, and hence on the mechanisms of interaction of laser radiation with biological tissue.

Practical Method for engineering Erbium-doped fiber lasers from step-like pulse excitations

International Nuclear Information System (INIS)

Causado-Buelvas, J D; Gomez-Cardona, N D; Torres, P

2011-01-01

A simple method, known as 'easy points', has been applied to the characterization of Erbium-doped fibers, aiming for the engineering of fiber lasers. Using low- optical-power flattop pulse excitations it has been possible to determine both the attenuation coefficients and the intrinsic saturation powers of doped single-mode fibers at 980 and 1550 nm. Laser systems have been projected for which the optimal fiber length and output power have been determined as a function of the input power. Ring and linear laser cavities have been set up, and the characteristics of the output laser have been obtained and compared with the theoretical predictions based on the 'easy points' parameters.

Pulse picker for synchrotron radiation driven by a surface acoustic wave.

Science.gov (United States)

Vadilonga, Simone; Zizak, Ivo; Roshchupkin, Dmitry; Petsiuk, Andrei; Dolbnya, Igor; Sawhney, Kawal; Erko, Alexei

2017-05-15

A functional test for a pulse picker for synchrotron radiation was performed at Diamond Light Source. The purpose of a pulse picker is to select which pulse from the synchrotron hybrid-mode bunch pattern reaches the experiment. In the present work, the Bragg reflection on a Si/B4C multilayer was modified using surface acoustic wave (SAW) trains. Diffraction on the SAW alters the direction of the x rays and it can be used to modulate the intensity of the x rays that reach the experimental chamber. Using electronic modulation of the SAW amplitude, it is possible to obtain different scattering conditions for different x-ray pulses. To isolate the single bunch, the state of the SAW must be changed in the short time gap between the pulses. To achieve the necessary time resolution, the measurements have been performed in conical diffraction geometry. The achieved time resolution was 120 ns.

Micro-pulses generation in ECR breakdown stimulated by gyrotron radiation at 37,5 GHz

International Nuclear Information System (INIS)

Skalyga, V.; Zorin, V.; Izotov, I.; Golubev, S.; Razin, S.; Sidorov, A.; Vodopyanov, A.

2012-01-01

The present work is devoted to experimental and theoretical investigation of the creation of short pulsed (< 100 μs) multicharged ion beams. The possibility of quasi-stationary generation of short pulsed beams under conditions of quasi-gasdynamic plasma confinement was shown in recent experiments. Later another way of such beams creation based on the Pre-glow effect was proposed. In present work it was demonstrated that in the case when duration of microwave (MW) pulse is less than formation time of Pre-glow peak, realization of a regime when ion current is negligible during MW pulse and intense multicharged ions flux appears only when MW ends could be possible. Such pulses after the end of MW were called micro-pulses. In the present work the generation of micro-pulses was observed in experiments with ECR discharge stimulated by gyrotron radiation at 37,5 GHz, 100 kW. In this case pulses with duration less than 30 μs were obtained. Probably the same effect was observed in GANIL where 14 GHz radiation was used and pulses with duration about 2 ms were registered. In present work it was shown that the intensity of such micro-pulse could be higher than intensity of Pre-glow peak at the same conditions but with longer MW pulse. The generation of micro-pulses of nitrogen and argon multicharged ions with current of a few mA and length about 30 μs after MW pulse with duration of 30-100 μs was demonstrated. The low level of impurities, high current density and rather high average charge make possible to consider such micro-pulse regime as a possibility for the creation of a short pulsed ion source. The paper is followed by the slides of the presentation. (authors)

Intersubband Rabi oscillations in asymmetric nanoheterostructures: implications for a tunable continuous-wave source of a far-infrared and THz radiation.

Science.gov (United States)

Kukushkin, V A

2012-06-01

A tunable continuous-wave source of a far-infrared and THz radiation based on a semiconductor nanoheterostructure with asymmetric quantum wells is suggested. It utilizes Rabi oscillations at a transition between quantum well subbands excited by external femtosecond pulses of a mid-infrared electromagnetic field. Due to quantum well broken inversion symmetry the subbands possess different average dipole moments, which enables the creation of polarization at the Rabi frequency as the subband populations change. It is shown that if this polarization is excited so that it is periodic in space, then, though being pulsed, it can produce continuous-wave output radiation. Changing the polarization space period and the time intervals between the exciting pulses, one can tune the frequency of this radiation throughout the far-infrared and THz range. In the present work a concrete multiple quantum well heterostructure design and a scheme of its space-periodic polarization are suggested. It is shown that for existing sources of mid-infrared femtosecond pulses the proposed scheme can provide a continuous-wave output power of order the power of far-infrared and THz quantum cascade lasers. Being added to the possibility of its output frequency tuning, this can make the suggested device attractive for fundamental research and various applications.

Accuracy of Analog Fiber-Optic Links in Pulsed Radiation Environments

International Nuclear Information System (INIS)

E K Miller; G S Macrum; I J McKenna

2007-01-01

Interferometric fiber-optic links used in pulsed-power experiments are evaluated for accuracy in the presence of radiation fields which alter fiber transmission. Amplitude-modulated format (e.g., Mach-Zehnder) and phase-modulated formats are compared. Historically, studies of radiation effects on optical fibers have focused on degradation and recovery of the fibers transmission properties; such work is either in the context of survivability of fibers in catastrophic conditions or suitability of fibers installed for command and control systems within an experimental facility [1], [2]. In this work, we consider links used to transmit realtime diagnostic data, and we analyze the error introduced by radiation effects during the drive pulse. The result is increased uncertainties in key parameters required to unfold the sinusoidal transfer function. Two types of modulation are considered: amplitude modulation typical of a Mach-Zehnder (M-Z) modulator [3], and phase modulation, which offers more flexible demodulation options but relies on the spatiotemporal coherence of the light in the fiber. The M-Z link is shown schematically in Fig. 1, and the phase-modulated link is shown in Fig. 2. We present data from two experimental environments: one with intense, controlled radiation fields to simulate conditions expected at the next generation of pulsed-power facilities, and the second with radiation effects below the noise level of the recording system. In the first case, we intentionally expose three types of single-mode fiber (SMF) to ionizing radiation and study the response by simultaneously monitoring phase and amplitude of the transmitted light. The phase and amplitude effects are evidently dominated by different physical phenomena, as their recovery dynamics are markedly different; both effects, though, show similar short-term behavior during exposure, integrating the dose at the dose levels studied, from 1 to 300 kRad, over the exposure times of 50 ps and 30 ns. In the

Pulse Splitting for Harmonic Beamforming in Time-Modulated Linear Arrays

Directory of Open Access Journals (Sweden)

Lorenzo Poli

2014-01-01

Full Text Available A novel strategy for harmonic beamforming in time-modulated linear arrays is proposed. The pulse splitting technique is exploited to simultaneously generate two harmonic patterns, one at the central frequency and another at a preselected harmonic of arbitrary order, while controlling the maximum level of the remaining sideband radiations. An optimization strategy based on the particle swarm optimizer is developed in order to determine the optimal parameters describing the pulse sequence used to modulate the excitation weights of the array elements. Representative numerical results are reported and discussed to point out potentialities and limitations of the proposed approach.

Modeling of collisional excited x-ray lasers using short pulse laser pumping

Energy Technology Data Exchange (ETDEWEB)

Sasaki, Akira; Moribayashi, Kengo; Utsumi, Takayuki; Tajima, Toshiki [Japan Atomic Energy Research Inst., Neyagawa, Osaka (Japan). Kansai Research Establishment

1998-03-01

A simple atomic kinetics model of electron collisional excited x-ray lasers has been developed. The model consists of a collisional radiative model using the average ion model (AIM) and a detailed term accounting (DTA) model of Ni-like Ta. An estimate of plasma condition to produce gain in Ni-like Ta ({lambda}=44A) is given. Use of the plasma confined in a cylinder is proposed to preform a uniform high density plasma from 1-D hydrodynamics calculations. (author)

Nonresonant Multiple-Pulse Control of Molecular Motions in Liquid

Directory of Open Access Journals (Sweden)

Nikiforov V.G.

2015-01-01

Full Text Available We propose the implementation of the multiple-pulse excitation for manipulation of the molecular contributions to the optically-heterodyne-detected optical-Kerr-effect. The key parameters controlling the specificity of the multiple-pulse excitation scenarios are the pulses durations, the delays between pulses, the relation between the pump pulses amplitudes and the pulses polarizations. We model the high-order optical responses and consider some principles of the scenarios construction. We show that it is possible to adjust the excitation scenario in such a way that the some responses can be removed from detected signal along with the enhancement of the interested response amplitude. The theoretical analysis and first experimental data reveal that the multiple-pulse excitation technique can be useful for the selective spectroscopy of the molecular vibrations and rotations in liquid.

Plasma focus - a pulsed radiation source

International Nuclear Information System (INIS)

Blagoev, Alexandar; Zapryanov, Stanislav; Gol'tsev, Vasilii; Gemishev, Orlin

2014-01-01

The article is devoted to the applications of plasma focus (PF) in radiobiology. Briefly describes the principle of operation of the device and the parameters of the PF type 'Mader' at the Physics Department of the University. Phase pinch discharge zones appear hot and dense plasma, which is a source of X-ray and neutron pulse when the working gas is deuterium. These radiations are essential for biological applications. Besides these bundles are obtained from accelerated charged particles and shock wave of ionized gas. Described are some of the contributions of other authors using PF in radiobiology. Given the results in the exposure of living organisms with soft X-ray emission of PF. We examined the viability of the cells of the two types of yeasts, after irradiation with X-rays at a dose of 65 mSv, where no change was found on the performance. It is shown that soft X-ray radiation doses on the order of tens of mSv, cause a significant change in the productivity of the electronic transport in the photosynthetic apparatus of Chlamydomonas reinhardtii. Trichoderma reesei M7 shows remarkable vitality irradiation with substantial doses of hard X-ray radiation (tens Sv). Appear endoglyukonazata changes in the protein component and the residual mass

Generation of pulsed far-infrared radiation and its application for far-infrared time-resolved spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Kondo, Yasuhiro [Tohoku Univ., Sendai (Japan). Faculty of Engineering

1996-07-01

So-called time-resolved spectroscopy technique has been used from old time as the means for studying the dynamic optical property, light-induced reaction and so on of matters. As an example, there is the method called pump and probe, and here, the wavelength of this probe light is the problem. If the object energy region is limited to about 0.1 eV, fast time-resolved spectroscopy is feasible relatively easily. However, energy region is extended to low energy region, the light source which is available as the pulsed probe light having sufficient intensity is limited. In this paper, the attempt of time-resolved spectroscopy utilizing coherent radiation, which has ended in failure, and the laser pulse-induced far-infrared radiation which can be utilized as new far-infrared probe light are reported. The reason why far-infrared radiation is used is explained. The attempt of time-resolved spectroscopy using NaCl crystals is reported on the equipment, the method of measuring absorption spectra and the results. Laser pulse-induced far-infrared radiation and the method of generating it are described. The multi-channel detector for far-infrared radiation which was made for trial is shown. (K.I.)

Effect of radiation damping on the interaction of ultra-intense laser pulses with an overdense plasma

International Nuclear Information System (INIS)

Zhidkov, Alexei; Koga, James; Sasaki, Akira; Ueshima, Yutaka

2001-01-01

The effect of radiation damping on the interaction of an ultra-intense laser pulse with an overdense plasma is studied via relativistic particle-in-cell simulation. The calculation is performed for a Cu solid slab including ionization. We find a strong effect from radiation damping on the electron energy cut-off at about 150 MeV and on the absorption of a laser pulse with an intensity I=5x10 22 W/cm 2 and duration of 20 fs. Hot electrons reradiate more then 10% of the laser energy during the laser pulse. With the laser intensity, the energy loss due to the radiation damping increases as I 3 . In addition, we observe that the laser pulse may not propagate in the plasma even if ω pl 2 /ω 2 γ<1. The increase of skin depth with the laser intensity due to relativistic effects gives rise to the absorption efficiency. (author)

Effects of excitation spectral width on decay profile of weakly confined excitons

International Nuclear Information System (INIS)

Kojima, O.; Isu, T.; Ishi-Hayase, J.; Kanno, A.; Katouf, R.; Sasaki, M.; Tsuchiya, M.

2008-01-01

We report the effect due to a simultaneous excitation of several exciton states on the radiative decay profiles on the basis of the nonlocal response of weakly confined excitons in GaAs thin films. In the case of excitation of single exciton state, the transient grating signal has two decay components. The fast decay component comes from nonlocal response, and the long-lived component is attributed to free exciton decay. With an increase of excitation spectral width, the nonlocal component becomes small in comparison with the long-lived component, and disappears under irradiation of a femtosecond-pulse laser with broader spectral width. The transient grating spectra clearly indicates the contribution of the weakly confined excitons to the signal, and the exciton line width hardly changes by excitation spectral width. From these results, we concluded that the change of decay profile is attributed not to the many-body effect but to the effect of simultaneous excitation of several exciton states

THE EXCITED LOADS OF ATTRACTION IN A SYMMETRICAL INDUCTOR SYSTEM FOR THE MAGNETIC PULSE REMOVING OF THE BODY CAR

Directory of Open Access Journals (Sweden)

A. V. Gnatov

2015-04-01

Full Text Available Recently, repair and recovery of vehicle body operations become more and more popular. A special place here is taken by equipment that provides performance of given repair operations. The most interesting are methods for recovery of car body panels that allow the straightening without disassembling of car body panels and damaging of existing protective coating. Now, there are several technologies for repair and recovery of car body panels without their disassembly and dismantling. The most perspective is magnetic-pulse technology of external noncontact straightening. Results. The calculation of excited loads attractions in a symmetrical inductor system in the universal tool of magnetic-pulse straightening is provided. According to the obtained analytical dependence of the numerical evaluation of volumetric construction diagrams, phase and amplitude of the radial dependence of the spatial distribution of the excited efforts of attraction is obtained. The influence of the magnetic properties of the blank screen and manifested in the appearance of powerful magnetic attraction forces is determined. Originality. A new trend of research of magnetic-pulse working of thin-walled metals has been formulated and received further development, which allows to create not only new equipment, but principally new technological processes of external non-contact repair and recovery of vehicle body panels. Scientific basis of electrodynamic and magnetic attraction of thin-walled sheet metals with using the energy of high-power pulsed fields was created for the first time and proved theoretically and experimentally. Scientific and technical solutions in design of effective tools based on single-turn inductor systems of cylindrical geometry for straightening and recovery of car body panels were formulated and proved theoretically, as well as experimentally. Practical value. Using the results of the calculations we can create effective tools for an external magnetic

Theory of propagation of spectrum and correlations of radiation in optically dense gas in the case of the closed excitation contour

International Nuclear Information System (INIS)

Barantsev, K.A.; Litvinov, A.N.; Popov, E.N.

2017-01-01

This work is devoted to generalization of the semi-classical theory of interaction of broadband laser radiation with the atomic gas at the room temperature in the cell in the case of the closed excitation contour. The atomic density matrix equations and spectrum and correlations transport equations have been derived for excitation by fluctuating field with Gaussian statistics. It is shown that the spatial oscillations of radiation intensity and atomic density matrix can be excited. It was found that such medium can serve as a filter of incoherent part of the radiation.

Spin gymnastics with selective radiofrequency pulses

Energy Technology Data Exchange (ETDEWEB)

Freeman, R.; Kupce, E. [Cambridge Univ. (United Kingdom)

1994-12-31

Although high resolution NMR spectra are normally excited with short intense radiofrequency pulses, there is an entire family of new experiments that can be performed with frequency-selective or ``soft`` pulses. Time-consuming two-dimensional spectroscopy may be reduced to a much shorter one-dimensional version with much finer digitization in the frequency domain. A large number of soft pulses can be combined to form a ``polychromatic pulse`` that has uniform excitation over the entire range of proton shifts except for a rejection notch at the water frequency. Polychromatic pulses can also be used to create antiphase magnetization in preparation for a coherence transfer or double-quantum experiment. An excitation profile can be designed in the form of a ``template`` that exactly matches the spectrum of a given chemical compound but has zero excitation elsewhere. This is achieved by using the information in the experimental free induction decay to construct a suitable array of soft pulses that has the required excitation pattern. In this manner, interpenetrating spectra can be separated into the spectra of the pure components, for example those of a and b glucose. Selective Hartmann-Hahn coherence transfer experiments employ similar soft pulse techniques. If several such transfers are concatenated, the method may be used as a test to see whether a group of protons is linked in an unbroken chain by scalar spin-spin interactions. (authors). 24 refs., 18 figs.

Femtosecond laser excitation of dielectric materials

DEFF Research Database (Denmark)

Wædegaard, Kristian Juncher; Balling, Peter; Frislev, Martin Thomas

2012-01-01

We report an approach to modeling the interaction between ultrashort laser pulses and dielectric materials. The model includes the excitation of carriers by the laser through strongfield excitation, collisional excitation, and absorption in the plasma consisting of conduction-band electrons formed...

Transient absorption spectroscopy in biology using the Super-ACO storage ring FEL and the synchrotron radiation combination

International Nuclear Information System (INIS)

Renault, Eric; Nahon, Laurent; Garzella, David; Nutarelli, Daniele; De Ninno, Giovanni; Hirsch, Matthias; Couprie, Marie Emmanuelle

2001-01-01

The Super-ACO storage ring FEL, covering the UV range down to 300 nm with a high average power (300 mW at 350 nm) together with a high stability and long lifetime, is a unique tool for the performance of users applications. We present here the first pump-probe two color experiments on biological species using a storage ring FEL coupled to the synchrotron radiation. The intense UV pulse of the Super-ACO FEL is used to prepare a high initial concentration of chromophores in their first singlet electronic excited state. The nearby bending magnet synchrotron radiation provides, on the other hand a pulsed, white light continuum (UV-IR), naturally synchronized with the FEL pulses and used to probe the photochemical subsequent events and the associated transient species. We have demonstrated the feasibility with a dye molecule (POPOP) observing a two-color effect, signature of excited state absorption and a temporal signature with Acridine. Applications on various chromophores of biological interest are carried out, such as the time-resolved absorption study of the first excited state of Acridine

Trapped electronic states in YAG crystal excited by femtosecond radiation

Energy Technology Data Exchange (ETDEWEB)

Zavedeev, E.V.; Kononenko, V.V.; Konov, V.I. [General Physics Institute of RAS, Moscow (Russian Federation); National Research Nuclear University MEPhI (Moscow Engineering Physics Institute), Moscow (Russian Federation)

2017-07-15

The excitation of an electronic subsystem of an yttrium aluminum garnet by 800 nm femtosecond radiation was studied theoretically and experimentally. The spatio-temporal dynamics of the refractive index (n) inside the beam waist was explored by means of the pump-probe interferometric technique with a submicron resolution. The observed increase in n indicated the formation of bound electronic states relaxed for ∝ 150 ps. We showed that the experimental data agreed with the computational simulation based on the numerical solution of the nonlinear Schroedinger equation only if these transient states were considered to arise from a direct light-induced process but not from the decay of radiatively generated free-electron-hole pairs. (orig.)

Electronic excitations and their effect on the interionic forces in simulations of radiation damage in metals

International Nuclear Information System (INIS)

Race, C P; Mason, D R; Sutton, A P

2009-01-01

Using time-dependent tight-binding simulations of radiation damage cascades in a model metal we directly investigate the nature of the excitations of a system of quantum mechanical electrons in response to the motion of a set of classical ions. We furthermore investigate the effect of these excitations on the attractive electronic forces between the ions. We find that the electronic excitations are well described by a Fermi-Dirac distribution at some elevated temperature, even in the absence of the direct electron-electron interactions that would be required in order to thermalize a non-equilibrium distribution. We explain this result in terms of the spectrum of characteristic frequencies of the ionic motion. Decomposing the electronic force into four well-defined components within the basis of instantaneous electronic eigenstates, we find that the effect of accumulated excitations in weakening the interionic bonds is mostly (95%) accounted for by a thermal model for the electronic excitations. This result justifies the use of the simplifying assumption of a thermalized electron system in simulations of radiation damage with an electronic temperature dependence and in the development of temperature-dependent classical potentials.

Electronic excitations and their effect on the interionic forces in simulations of radiation damage in metals.

Science.gov (United States)

Race, C P; Mason, D R; Sutton, A P

2009-03-18

Using time-dependent tight-binding simulations of radiation damage cascades in a model metal we directly investigate the nature of the excitations of a system of quantum mechanical electrons in response to the motion of a set of classical ions. We furthermore investigate the effect of these excitations on the attractive electronic forces between the ions. We find that the electronic excitations are well described by a Fermi-Dirac distribution at some elevated temperature, even in the absence of the direct electron-electron interactions that would be required in order to thermalize a non-equilibrium distribution. We explain this result in terms of the spectrum of characteristic frequencies of the ionic motion. Decomposing the electronic force into four well-defined components within the basis of instantaneous electronic eigenstates, we find that the effect of accumulated excitations in weakening the interionic bonds is mostly (95%) accounted for by a thermal model for the electronic excitations. This result justifies the use of the simplifying assumption of a thermalized electron system in simulations of radiation damage with an electronic temperature dependence and in the development of temperature-dependent classical potentials.

Structure of picosecond pulses of a Q-switched and mode-locked diode-pumped Nd:YAG laser

Energy Technology Data Exchange (ETDEWEB)

Donin, V I; Yakovin, D V; Gribanov, A V [Institute of Automation and Electrometry, Siberian Branch of the Russian Academy of Sciences, Novosibirsk (Russian Federation)

2015-12-31

The pulse duration of a diode-pumped Nd:YAG laser, in which Q-switching with mode-locking (QML regime) is achieved using a spherical mirror and a travelling-wave acousto-optic modulator, is directly measured with a streak camera. It is found that the picosecond pulses can have a non-single-pulse structure, which is explained by excitation of several competing transverse modes in the Q-switching regime with a pulse repetition rate of 1 kHz. In the case of cw mode-locking (without Q-switching), a new (auto-QML) regime is observed, in which the pulse train repetition rate is determined by the frequency of the relaxation oscillations of the laser field while the train contains single picosecond pulses. (control of laser radiation parameters)

Parametric excitation electromagnetic radiation in a bounded non-equilibrium plasma

International Nuclear Information System (INIS)

Balakirev, V.A.; Tolstoluzhskij, A.P.

1981-01-01

An excitation mechanism of electromagnetic radiation in a bounded plasma-beam system which is based on the process of induced scattering of electron beam-strengthened high-frequency wave (HF) of a plasma waveguide with an ion-sound wave, is investigated. It is shown that the process under investigation is an effective mechanism of electromagnetic radiation production. Up to 73 % of the beam power is trabsformed to the electromagnetic radiation under the conditions considered. As the frequency of the irradiated wave is close to the plasma frequency it can vary within wide limits by the change in plasma density. It is noted that the necessary condition of electromagnetic radiation production in the mechanism under consideration has the form of inequality ωsub(l)-ωsub(s)/(ksub(l)-ksub(s)>c (ωsub(l) - frequency of HF wave, ωsub(s)- frequency of ion-sound wave) and is less rigid as compared with the synchronism conditions for three-wave resonant interaction of proper oscillations. Therefore, the considered induced scattering process is less sensitive to a possible inhomogeneity of plasma density [ru

Switching Exciton Pulses Through Conical Intersections

Science.gov (United States)

Leonhardt, K.; Wüster, S.; Rost, J. M.

2014-11-01

Exciton pulses transport excitation and entanglement adiabatically through Rydberg aggregates, assemblies of highly excited light atoms, which are set into directed motion by resonant dipole-dipole interaction. Here, we demonstrate the coherent splitting of such pulses as well as the spatial segregation of electronic excitation and atomic motion. Both mechanisms exploit local nonadiabatic effects at a conical intersection, turning them from a decoherence source into an asset. The intersection provides a sensitive knob controlling the propagation direction and coherence properties of exciton pulses. The fundamental ideas discussed here have general implications for excitons on a dynamic network.

Continuous micro-feeding of fine cohesive powders actuated by pulse inertia force and acoustic radiation force in ultrasonic standing wave field.

Science.gov (United States)

Wang, Hongcheng; Wu, Liqun; Zhang, Ting; Chen, Rangrang; Zhang, Linan

2018-07-10

Stable continuous micro-feeding of fine cohesive powders has recently gained importance in many fields. However, it remains a great challenge in practice because of the powder aggregate caused by interparticle cohesive forces in small capillaries. This paper describes a novel method of feeding fine cohesive powder actuated by a pulse inertia force and acoustic radiation force simultaneously in an ultrasonic standing wave field using a tapered glass nozzle. Nozzles with different outlet diameters are fabricated using glass via a heating process. A pulse inertia force is excited to drive powder movement to the outlet section of the nozzle in a consolidated columnar rod mode. An acoustic radiation force is generated to suspend the particles and make the rod break into large quantities of small agglomerates which impact each other randomly. So the aggregation phenomenon in the fluidization of cohesive powders can be eliminated. The suspended powder is discharged continuously from the nozzle orifice owing to the self-gravities and collisions between the inner particles. The micro-feeding rates can be controlled accurately and the minimum values for RespitoseSV003 and Granulac230 are 0.4 mg/s and 0.5 mg/s respectively. The relative standard deviations of all data points are below 0.12, which is considerably smaller than those of existing vibration feeders with small capillaries. Copyright © 2018 Elsevier B.V. All rights reserved.

Stable radiation pressure acceleration of ions by suppressing transverse Rayleigh-Taylor instability with multiple Gaussian pulses

Energy Technology Data Exchange (ETDEWEB)

Zhou, M. L.; Liu, B.; Hu, R. H.; Shou, Y. R.; Lin, C.; Lu, H. Y.; Lu, Y. R.; Ma, W. J., E-mail: wenjun.ma@pku.edu.cn [State Key Laboratory of Nuclear Physics and Technology, and Key Laboratory of HEDP of the Ministry of Education, CAPT, Peking University, Beijing 100871 (China); Gu, Y. Q. [Laser Fusion Research Center, China Academy of Engineering Physics, Mianyang, Sichuan 621900 (China); Yan, X. Q., E-mail: x.yan@pku.edu.cn [State Key Laboratory of Nuclear Physics and Technology, and Key Laboratory of HEDP of the Ministry of Education, CAPT, Peking University, Beijing 100871 (China); Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, Shanxi 030006 (China)

2016-08-15

In the case of a thin plasma slab accelerated by the radiation pressure of an ultra-intense laser pulse, the development of Rayleigh-Taylor instability (RTI) will destroy the acceleration structure and terminate the acceleration process much sooner than theoretical limit. In this paper, a new scheme using multiple Gaussian pulses for ion acceleration in a radiation pressure acceleration regime is investigated with particle-in-cell simulation. We found that with multiple Gaussian pulses, the instability could be efficiently suppressed and the divergence of the ion bunch is greatly reduced, resulting in a longer acceleration time and much more collimated ion bunch with higher energy than using a single Gaussian pulse. An analytical model is developed to describe the suppression of RTI at the laser-plasma interface. The model shows that the suppression of RTI is due to the introduction of the long wavelength mode RTI by the multiple Gaussian pulses.

Electronic and structural response of nanomaterials to ultrafast and ultraintense laser pulses.

Science.gov (United States)

Jiang, Chen-Wei; Zhou, Xiang; Lin, Zhibin; Xie, Rui-Hua; Li, Fu-Li; Allen, Roland E

2014-02-01

The interaction of materials with ultrafast and ultraintense laser pulses is a current frontier of science both experimentally and theoretically. In this review, we briefly discuss some recent theoretical studies by the present authors with our method of semiclassical electron-radiation-ion dynamics (SERID). In particular, Zhou et al. and Jiang et al. respectively, determined the optimal duration and optimal timing for a series of femtosecond scale laser pulses to excite a specific vibrational mode in a general chemical system. A set of such modes can be used as a "fingerprint" for characterizing a particular molecule or a complex in a solid. One can therefore envision many applications, ranging from fundamental studies to detection of chemical or biological agents. Allen et al. proved that dimers are preferentially emitted during photofragmentation of C60 under an ultrafast and ultraintense laser pulse. For interactions between laser pulses and semiconductors, e.g., GaAs, Si and InSb, besides experimentally accessible optical properties--epsilon(omega) and chi(2)-Allen et al. offered many other indicators to confirm the nonthermal nature of structural changes driven by electronic excitations and occurring during the first few hundred femtoseconds. Lin et al. found that, after the application of a femtosecond laser pulse, excited electrons in materials automatically equilibrate to a Fermi-Dirac distribution within roughly 100 fs, solely because of their coupling to the nuclear motion, even though the resulting electronic temperature is one to two orders of magnitude higher than the kinetic temperature defined by the nuclear motion.

Conductivity of ion dielectrics during the mean flux-density electron- and X-ray pulse radiation

International Nuclear Information System (INIS)

Vajsburd, D.I.; Mesyats, G.A.; Naminov, V.L.; Tavanov, Eh.G.

1982-01-01

Conductivity of ion dielectrics under electron and X-ray pulse radiation is investigated. Investigations have been conducted in the range of average beam densities in which extinction of low-energy conductivity takes place. Thin plates of alkali-halogen crystals have been used as samples. Small-dimensional accelerator with controlled beam parameters: 1-20 ns, 0.1-2000 A/cm 2 , 0.3-0.5 MeV has been used for radiation. Temperature dependence of conductivity current pulse is determined. Time resolution of 10 - 10 s is achieved. In the 70-300 K range it practically coincides with radiation pulse. An essential inertial constituent is observed below 300 K. It is shown that at average beam densities a comparable contribution into fast conductivity is made by intracentre conductivity independent of temperature and high-temperature conductivity which decreases with temperature with activation energy equal to the energy of short-wave background. That is why amplitude of fast constituent decreases with temperature slower than high-energy conductivity

High power laser exciter accelerators

International Nuclear Information System (INIS)

Martin, T.H.

1975-01-01

Recent developments in untriggered oil and water switching now permit the construction of compact, high energy density pulsed power sources for laser excitation. These accelerators, developed principally for electron beam fusion studies, appear adaptable to laser excitation and will provide electron beams of 10 13 to 10 14 W in the next several years. The accelerators proposed for e-beam fusion essentially concentrate the available power from the outside edge of a disk into the central region where the electron beam is formed. One of the main problem areas, that of power flow at the vacuum diode insulator, is greatly alleviated by the multiplicity of electron beams that are allowable for laser excitation. A proposal is made whereby the disk-shaped pulsed power sections are stacked vertically to form a series of radially flowing electron beams to excite the laser gas volume. (auth)

Method for detecting and distinguishing between specific types of environmental radiation using a high pressure ionization chamber with pulse-mode readout

Science.gov (United States)

Degtiarenko, Pavel V.

2017-12-19

An environmental radiation detector for detecting and distinguishing between all types of environmental radiation, including photons, charged particles, and neutrons. A large volume high pressure ionization chamber (HPIC) includes BF.sub.3 gas at a specific concentration to render the radiation detector sensitive to the reactions of neutron capture in Boron-10 isotope. A pulse-mode readout is connected to the ionization chamber capable of measuring both the height and the width of the pulse. The heavy charged products of the neutron capture reaction deposit significant characteristic energy of the reaction in the immediate vicinity of the reaction in the gas, producing a signal with a pulse height proportional to the reaction energy, and a narrow pulse width corresponding to the essentially pointlike energy deposition in the gas. Readout of the pulse height and the pulse width parameters of the signals enables distinguishing between the different types of environmental radiation, such as gamma (x-rays), cosmic muons, and neutrons.

INTERACTION OF LASER RADIATION WITH MATTER: Influence of surface breakdown on the process of drilling metals with pulsed CO2 laser radiation

Science.gov (United States)

Arutyunyan, R. V.; Baranov, V. Yu; Bobkov, I. V.; Bol'shov, Leonid A.; Dolgov, V. A.; Kanevskiĭ, M. F.; Malyuta, D. D.; Mezhevov, V. S.

1988-03-01

A report is given of the influence of low-threshold surface optical breakdown, occurring under the action of short (~ 5-μs) radiation pulses from a CO2 laser, on the process of the laser drilling of metals. Data are given on the difference between the interaction of radiation pulses having the same duration but differing in shape. A study was made of the influence of the pressure of the atmosphere surrounding a target on the results of laser drilling of metals. A theoretical explanation is given of the experimental results.

Evaluation of material dispersion using a nanosecond optical pulse radiator.

Science.gov (United States)

Horiguchi, M; Ohmori, Y; Miya, T

1979-07-01

To study the material dispersion effects on graded-index fibers, a method for measuring the material dispersion in optical glass fibers has been developed. Nanosecond pulses in the 0.5-1.7-microm region are generated by a nanosecond optical pulse radiator and grating monochromator. These pulses are injected into a GeO(2)-P(2)0(5)-doped silica graded-index fiber. Relative time delay changes between different wavelengths are used to determine material dispersion, core glass refractive index, material group index, and optimum profile parameter of the graded-index fiber. From the measured data, the optimum profile parameter on the GeO(2)-P(2)O(5)-doped silica graded-index fiber could be estimated to be 1.88 at 1.27 microm of the material dispersion free wavelength region and 1.82 at 1.55 microm of the lowest-loss wavelength region in silica-based optical fiber waveguides.

Short-Lived Electronically-Excited Diatomic Molecules Cooled via Supersonic Expansion from a Plasma Microjet

Science.gov (United States)

Houlahan, Thomas J., Jr.; Su, Rui; Eden, Gary

2014-06-01

Using a pulsed plasma microjet to generate short-lived, electronically-excited diatomic molecules, and subsequently ejecting them into vacuum to cool via supersonic expansion, we are able to monitor the cooling of molecules having radiative lifetimes as low as 16 ns. Specifically, we report on the rotational cooling of He_2 molecules in the d^3Σ_u^+, e^3Π_g, and f^3Σ_u^+ states, which have lifetimes of 25 ns, 67 ns, and 16 ns, respectively. The plasma microjet is driven with a 2.6 kV, 140 ns high-voltage pulse (risetime of 20 ns) which, when combined with a high-speed optical imaging system, allows the nonequilibrium rotational distribution for these molecular states to be monitored as they cool from 1200 K to below 250 K with spatial and temporal resolutions of below 10 μm and 10 ns, respectively. The spatial and temporal resolution afforded by this system also allows the observation of excitation transfer between the f^3Σ_u^+ state and the lower lying d^3Σ_u^+ and e^3Π_g states. The extension of this method to other electronically excited diatomics with excitation energies >5 eV will also be discussed.

Molecular spinning by a chiral train of short laser pulses

Science.gov (United States)

Floß, Johannes; Averbukh, Ilya Sh.

2012-12-01

We provide a detailed theoretical analysis of molecular rotational excitation by a chiral pulse train, a sequence of linearly polarized pulses with the polarization direction rotating from pulse to pulse by a controllable angle. Molecular rotation with a preferential rotational sense (clockwise or counterclockwise) can be excited by this scheme. We show that the directionality of the rotation is caused by quantum interference of different excitation pathways. The chiral pulse train is capable of selective excitation of molecular isotopologs and nuclear spin isomers in a mixture. We demonstrate this using 14N2 and 15N2 as examples for isotopologs and para- and ortho-nitrogen as examples for nuclear-spin isomers.

Spatial resolution and maximum compensation factor of two-dimensional selective excitation pulses for MRI of objects containing conductive implants

Directory of Open Access Journals (Sweden)

Taeseong Woo

2017-05-01

Full Text Available A quantitative diagnosis using magnetic resonance imaging (MRI can be disturbed by radiofrequency (RF field inhomogeneity induced by the conductive implants. This inhomogeneity causes a local decrease of the signal intensity around the conductor, resulting in a deterioration of the accurate quantification. In a previous study, we developed an MRI imaging method using a two-dimensional selective excitation pulse (2D pulse to mitigate signal inhomogeneity induced by metallic implants. In this paper, the effect of 2D pulse was evaluated quantitatively by numerical simulation and MRI experiments. We introduced two factors for evaluation, spatial resolution and maximum compensation factor. Numerical simulations were performed with two groups. One group was composed of four models with different signal loss width, to evaluate the spatial resolution of the 2D pulse. The other group is also composed of four models with different amounts of signal loss for evaluating maximum compensation factor. In MRI experiments, we prepared phantoms containing conductors, which have different electrical conductivities related with the amounts of signal intensity decrease. The recovery of signal intensity was observed by 2D pulses, in both numerical simulations and experiments.

Optimal initiation of electronic excited state mediated intramolecular H-transfer in malonaldehyde by UV-laser pulses

Science.gov (United States)

Nandipati, K. R.; Singh, H.; Nagaprasad Reddy, S.; Kumar, K. A.; Mahapatra, S.

2014-12-01

Optimally controlled initiation of intramolecular H-transfer in malonaldehyde is accomplished by designing a sequence of ultrashort (~80 fs) down-chirped pump-dump ultra violet (UV)-laser pulses through an optically bright electronic excited [ S 2 ( π π ∗)] state as a mediator. The sequence of such laser pulses is theoretically synthesized within the framework of optimal control theory (OCT) and employing the well-known pump-dump scheme of Tannor and Rice [D.J. Tannor, S.A. Rice, J. Chem. Phys. 83, 5013 (1985)]. In the OCT, the control task is framed as the maximization of cost functional defined in terms of an objective function along with the constraints on the field intensity and system dynamics. The latter is monitored by solving the time-dependent Schrödinger equation. The initial guess, laser driven dynamics and the optimized pulse structure (i.e., the spectral content and temporal profile) followed by associated mechanism involved in fulfilling the control task are examined in detail and discussed. A comparative account of the dynamical outcomes within the Condon approximation for the transition dipole moment versus its more realistic value calculated ab initio is also presented.

Luminescence decay of S Zn::Ag and O Zn:Ga scintillation detectors excited by a pulsed laser

International Nuclear Information System (INIS)

Romero, L.; Campos, J.

1981-01-01

In the present work a high sensitivity experimental set up for luminescence decay measurements in the 1 0 - 1 sec range has been developed. As an application, luminescence light decay In S Zn:Ag and 0Zn:Ga after excitation by a pulsed N 2 laser has been measured. In SZnrAg, measurements of total light decay was compared with donor acceptor pairs theory. In both substances, spectral evolution in the first 15 sec was investigated. (Author) 4 refs

Studies on the transmission and processing of pulse-shaped signals from nuclear radiation detectors using methods of systems theory

International Nuclear Information System (INIS)

Spillekothen, H.G.

2007-01-01

Using methods of the systems theory of electronic communications and theoretical electrical science, this study describes the transmission of pulse-shaped signals from nuclear radiation detectors from the detector over ''electrically long lines'' (cables) to the output of the first pulse amplifier. The example of pulses from BF 3 -proportional counters shows, using the Fourier transformation, that pulses from radiation detectors contain a frequency spectrum ranging well above 10 8 Hz. If these pulses are transmitted to the first amplifier over a line length of several meters, the laws of the theory of transmission lines must be taken into account to avoid false signals caused by reflections. In the example, line equations are applied and the influence of the line and the terminating impedance is demonstrated. The influence of the frequency response ν(ω) and the phase response δ(ω) of the amplifier is also considered in the sample calculation. The methods presented make it possible to analyze and optimize the transmission and amplification of signals from radiation detectors. Close agreement emerges between empirically observed and calculated pulse shapes. (orig.)

Energy-optimal electrical excitation of nerve fibers.

Science.gov (United States)

Jezernik, Saso; Morari, Manfred

2005-04-01

We derive, based on an analytical nerve membrane model and optimal control theory of dynamical systems, an energy-optimal stimulation current waveform for electrical excitation of nerve fibers. Optimal stimulation waveforms for nonleaky and leaky membranes are calculated. The case with a leaky membrane is a realistic case. Finally, we compare the waveforms and energies necessary for excitation of a leaky membrane in the case where the stimulation waveform is a square-wave current pulse, and in the case of energy-optimal stimulation. The optimal stimulation waveform is an exponentially rising waveform and necessitates considerably less energy to excite the nerve than a square-wave pulse (especially true for larger pulse durations). The described theoretical results can lead to drastically increased battery lifetime and/or decreased energy transmission requirements for implanted biomedical systems.

Zeeman effect on disalignment of excited atoms by radiation re-absorption: neon 2p2 atoms in a discharge plasma

International Nuclear Information System (INIS)

Deguchi, K; Imagawa, T; Shikama, T; Hasuo, M

2009-01-01

We have measured the relaxation rate of alignment of neon atoms in a 2p 2 (in Paschen notation) level, which were excited by a linearly polarized laser pulse in a glow discharge plasma at 77 K, in a magnetic field of up to 3 T in the Voigt configuration. The relaxation rate decreased with an increase in the magnetic field strength of up to 0.5 T and showed no magnetic field dependence above 0.5 T. We developed a Monte Carlo simulation method to calculate alignment relaxation, or disalignment, by radiation re-absorption of atomic resonance lines in a magnetic field. The simulated result was found to be consistent with the observed magnetic field dependence. We analysed the results of the simulation from a point of competition between the Zeeman splitting and the Doppler broadening of the transition lines from the 2p 2 level.

Pulse radiation effects in high temperature superconductors. [YBaCuO

Energy Technology Data Exchange (ETDEWEB)

Korenev, S.A. (Joint Inst. for Nuclear Research, Dubna (Russia))

1992-03-01

Radiation effects in high temperature superconducting (HTSC) films, influenced by pulse electron and ion beams, are considered. The electron beams had kinetic energies E = 200-300 keV, current densities j = 10-2000 A/cm{sup 2} and pulse duration t{sub p} = 0.3-1.2 {mu}s; and ion beams of carbon, copper and silver with E = 200-350 keV, t{sub p} = 0.3 {mu}s and j = 5-15 A/cm{sup 2} were used in the experiments. The results of resistive threshold characteristics measurements by HTSC are described. Questions about the increase of critical current and electric strength of vacuum gaps with electrodes from HTSC are discussed. (orig.).

Interaction of Repetitively Pulsed High Energy Laser Radiation With Matter

Science.gov (United States)

Hugenschmidt, Manfred

1986-10-01

The paper is concerned with laser target interaction processes involving new methods of improving the overall energy balance. As expected theoretically, this can be achieved with high repetition rate pulsed lasers even for initially highly reflecting materials, such as metals. Experiments were performed by using a pulsed CO2 laser at mean powers up to 2 kW and repetition rates up to 100 Hz. The rates of temperature rise of aluminium for example were thereby increased by lore than a factor of 3 as compared to cw-radiation of comparable power density. Similar improvements were found for the overall absorptivities that were increased by this method by more than an order of magnitude.

Excitation of high energy levels under laser exposure of suspensions of nanoparticles in liquids

Energy Technology Data Exchange (ETDEWEB)

Shafeev, G.A. [Wave Research Center of A.M. Prokhorov General Physics Institute, 38, Vavilov Street, 119991 Moscow (Russian Federation)], E-mail: shafeev@kapella.gpi.ru; Simakin, A.V. [Wave Research Center of A.M. Prokhorov General Physics Institute, 38, Vavilov Street, 119991 Moscow (Russian Federation); Bozon-Verduraz, F. [ITODYS, UMR CNRS 7086, Universite Paris 7-Denis Diderot, 2, place Jussieu, 75251 Paris cedex 05 (France); Robert, M. [Laboratoire d' Electrochimie Moleculaire, UMR CNRS 7591, Universite Paris 7 Denis Diderot, 2, place Jussieu, 75251 Paris cedex 05 (France)

2007-12-15

Laser exposure of suspensions of nanoparticles in liquids leads to excitation of high energy levels in both liquid and nanoparticle material. The emission spectrum of the colloidal solution under exposure of a suspension metallic nanoparticles in water to radiation of a Nd:YAG laser of a picosecond range of pulse duration is discussed. Excitation of nuclear energy levels and neutron release is experimentally studied on the model system of transmutation of Hg into Au that occurs under exposure of Hg nanodrops suspended in D{sub 2}O. The proposed mechanism involves: (i) emission of X-ray photons by Hg nanoparticles upon laser exposure, leading to neutron release from D{sub 2}O, (ii) initiation of Hg {yields} Au transmutation by the capture of neutrons. The effect of transmutation is more pronounced using {sup 196}Hg isotope instead of Hg of natural isotope composition. The influence of laser pulse duration on the degree of transmutation (from fs through ns range) is discussed.

Principles and techniques of radiation hardening. Volume 3. Electromagnetic pulse (EMP) and system generated EMP

International Nuclear Information System (INIS)

Rudie, N.J.

1976-01-01

The three-volume book is intended to serve as a review of the effects of thermonuclear explosion induced radiation (x-rays, gamma rays, and beta particles) and the resulting electromagnetic pulse (EMP). Volume 3 deals with the following topics: selected fundamentals of electromagnetic theory; EMP induced currents on antennas and cables; the EMP response of electronics; EMP hardening; EMP testing; injection currents; internal electromagnetic pulse (IEMP); replacement currents; and system generated electromagnetic pulse (SGEMP) hardening

Cavitation and shock waves emission on the rigid boundary of water under mid-IR nanosecond laser pulse excitation

Science.gov (United States)

Pushkin, A. V.; Bychkov, A. S.; Karabutov, A. A.; Potemkin, F. V.

2018-06-01

The processes of conversion of light energy into mechanical energy under mid-IR nanosecond laser excitation on a rigid boundary of water are investigated. Strong water absorption of Q-switched Cr:Yb:Ho:YSGG (2.85 µm, 6 mJ, 45 ns) laser radiation provides rapid energy deposition of ~8 kJ cm‑3 accompanied with strong mechanical transients. The evolution of shock waves and cavitation bubbles is studied using the technique of shadowgraphy and acoustic measurements, and the conversion efficiency into these energy channels for various laser fluence (0.75–2.0 J cm‑2) is calculated. For 6 mJ laser pulse with fluence of 2.0 J cm‑2, the conversion into shock wave energy reaches 67%. The major part of the shock wave energy (92%) is dissipated when the shock front travels the first 250 µm, and the remaining 8% is transferred to the acoustic far field. The calculated pressure in the vicinity of water-silicon interface is 0.9 GPa. Cavitation efficiency is significantly less and reaches up to 5% of the light energy. The results of the current study could be used in laser parameters optimization for micromachining and biological tissue ablation.

A pulsed plasma jet with the various Ar/N2 mixtures

Science.gov (United States)

Barkhordari, A.; Ganjovi, A.; Mirzaei, I.; Falahat, A.; Rostami Ravari, M. N.

2017-12-01

In this paper, using the Optical Emission Spectroscopy technique, the physical properties of a fabricated pulsed DBD plasma jet are studied. Ar/N2 gaseous mixture is taken as operational gas, and Ar contribution in Ar/N2 mixture is varied from 75 to 95%. Through the optical emission spectra analysis of the pulsed DBD plasma jet, the rotational, vibrational and excitation temperatures and density of electrons in plasma medium of the pulsed plasma jet are obtained. It is seen that, at the wavelength of 750.38 nm, the radiation intensity from the Ar 4p → 4 s transition increases at the higher Ar contributions in Ar/N2 mixture. It is found that, for 95% of Ar presence in the mixture, the emission intensities from argon and molecular nitrogen are higher, and the emission line intensities will increase nonlinearly. In addition, it is observed that the quenching of Ar* by N2 results in the higher intensities of N2 excited molecules. Moreover, at the higher percentages of Ar in Ar/N2 mixture, while all the plasma temperatures are increased, the plasma electron density is reduced.

Transient absorption spectroscopy in biology using the Super-ACO storage ring FEL and the synchrotron radiation combination

CERN Document Server

Renault, E; De Ninno, G; Garzella, D; Hirsch, M; Nahon, L; Nutarelli, D

2001-01-01

The Super-ACO storage ring FEL, covering the UV range down to 300 nm with a high average power (300 mW at 350 nm) together with a high stability and long lifetime, is a unique tool for the performance of users applications. We present here the first pump-probe two color experiments on biological species using a storage ring FEL coupled to the synchrotron radiation. The intense UV pulse of the Super-ACO FEL is used to prepare a high initial concentration of chromophores in their first singlet electronic excited state. The nearby bending magnet synchrotron radiation provides, on the other hand a pulsed, white light continuum (UV-IR), naturally synchronized with the FEL pulses and used to probe the photochemical subsequent events and the associated transient species. We have demonstrated the feasibility with a dye molecule (POPOP) observing a two-color effect, signature of excited state absorption and a temporal signature with Acridine. Applications on various chromophores of biological interest are carried out,...

TH-F-202-00: MRI for Radiation Therapy

International Nuclear Information System (INIS)

2016-01-01

MRI has excellent soft tissue contrast and can provide both anatomical and physiological information. It is becoming increasingly important in radiation therapy for treatment planning, image-guided radiation therapy, and treatment assessment. It is critically important at this time point to educate and update our medical physicists about MRI to prepare for the upcoming surge of MRI applications in radiation therapy. This session will review important basics of MR physics, pulse sequence designs, and current radiotherapy application, as well as showcase exciting new developments in MRI that can be potentially useful in radiation therapy. Learning Objectives: To learn basics of MR physics and understand the differences between various pulse sequences To review current applications of MRI in radiation therapy.To discuss recent MRI advances for future MRI guided radiation therapy Partly supported by NIH (1R21CA165384).; W. Miller, Research supported in part by Siemens Healthcare; G. Li, My clinical research is in part supported by NIH U54CA137788. I have a collaborative research project with Philips Healthcare.; J. Cai, jing cai

TH-F-202-00: MRI for Radiation Therapy

Energy Technology Data Exchange (ETDEWEB)

NONE

2016-06-15

MRI has excellent soft tissue contrast and can provide both anatomical and physiological information. It is becoming increasingly important in radiation therapy for treatment planning, image-guided radiation therapy, and treatment assessment. It is critically important at this time point to educate and update our medical physicists about MRI to prepare for the upcoming surge of MRI applications in radiation therapy. This session will review important basics of MR physics, pulse sequence designs, and current radiotherapy application, as well as showcase exciting new developments in MRI that can be potentially useful in radiation therapy. Learning Objectives: To learn basics of MR physics and understand the differences between various pulse sequences To review current applications of MRI in radiation therapy.To discuss recent MRI advances for future MRI guided radiation therapy Partly supported by NIH (1R21CA165384).; W. Miller, Research supported in part by Siemens Healthcare; G. Li, My clinical research is in part supported by NIH U54CA137788. I have a collaborative research project with Philips Healthcare.; J. Cai, jing cai.

Femtosecond pulse laser notch shaping via fiber Bragg grating for the excitation source on the coherent anti-Stokes Raman spectroscopy

Science.gov (United States)

Oh, Seung Ryeol; Kwon, Won Sik; Kim, Jin Hwan; Kim, Kyung-Soo; Kim, Soohyun

2015-03-01

Single-pulse coherently controlled nonlinear Raman spectroscopy is the simplest method among the coherent anti-Stokes Raman spectroscopy systems. In recent research, it has been proven that notch-shaped femtosecond pulse laser can be used to collect the coherent anti-Stokes Raman signals. In this study, we applied a fiber Bragg grating to the notch filtering component on the femtosecond pulse lasers. The experiment was performed incorporating a titanium sapphire femtosecond pulse laser source with a 100 mm length of 780-HP fiber which is inscribed 30 mm of Bragg grating. The fiber Bragg grating has 785 nm Bragg wavelength with 0.9 nm bandwidth. We proved that if the pulse lasers have above a certain level of positive group delay dispersion, it is sufficient to propagate in the fiber Bragg grating without any spectral distortion. After passing through the fiber Bragg grating, the pulse laser is reflected on the chirped mirror for 40 times to make the transform-limited pulse. Finally, the pulse time duration was 37 fs, average power was 50mW, and showed an adequate notch shape. Furthermore, the simulation of third order polarization signal is performed using MATLAB tools and the simulation result shows that spectral characteristic and time duration of the pulse is sufficient to use as an excitation source for single-pulse coherent anti-Stokes Raman spectroscopy. In conclusion, the proposed method is more simple and cost-effective than the methods of previous research which use grating pairs and resonant photonic crystal slab.

Simultaneous time-space resolved reflectivity and interferometric measurements of dielectrics excited with femtosecond laser pulses

Science.gov (United States)

Garcia-Lechuga, M.; Haahr-Lillevang, L.; Siegel, J.; Balling, P.; Guizard, S.; Solis, J.

2017-06-01

Simultaneous time-and-space resolved reflectivity and interferometric measurements over a temporal span of 300 ps have been performed in fused silica and sapphire samples excited with 800 nm, 120 fs laser pulses at energies slightly and well above the ablation threshold. The experimental results have been simulated in the frame of a multiple-rate equation model including light propagation. The comparison of the temporal evolution of the reflectivity and the interferometric measurements at 400 nm clearly shows that the two techniques interrogate different material volumes during the course of the process. While the former is sensitive to the evolution of the plasma density in a very thin ablating layer at the surface, the second yields an averaged plasma density over a larger volume. It is shown that self-trapped excitons do not appreciably contribute to carrier relaxation in fused silica at fluences above the ablation threshold, most likely due to Coulomb screening effects at large excited carrier densities. For both materials, at fluences well above the ablation threshold, the maximum measured plasma reflectivity shows a saturation behavior consistent with a scattering rate proportional to the plasma density in this fluence regime. Moreover, for both materials and for pulse energies above the ablation threshold and delays in the few tens of picoseconds range, a simultaneous "low reflectivity" and "low transmission" behavior is observed. Although this behavior has been identified in the past as a signature of femtosecond laser-induced ablation, its origin is alternatively discussed in terms of the optical properties of a material undergoing strong isochoric heating, before having time to substantially expand or exchange energy with the surrounding media.

The extreme condition analyzing for NEMPI shielding of electronic system in high-intensity pulsed radiation diagnosing

International Nuclear Information System (INIS)

Cheng Xiaolei; Liu Fang; Ouyang Xiaoping

2012-01-01

The difficulty for estimating the NEMPI (electromagnetic pulsed interference caused by the nuclear reaction) on the electronic system in high-intensity pulsed radiation diagnosing is analyzed in this article. To solve the difficulty, a method called 'Extreme Condition Analyzing' is presented for estimating the NEMPI conservatively and reliably. Through an extreme condition hypothesizing which could be described as 'Entire Coupling of Electric Field Energy', the E max (maximum electric field intensity which could be endured by the electronic system in the high-intensity pulsed radiation) could be figured out without any other information of the EMP caused by the nuclear reaction. Then a feasibility inspection is introduced, to confirm that the EMPI shielding request according to E max is not too extreme to be achieved. (authors)

P 8: Table-top instrumentation for time-resolved luminescence spectroscopy of solids excited by soft X-ray from a laser induced plasma source and/or UV-VIS laser

International Nuclear Information System (INIS)

Bruza, P.; Fidler, V.; Nikl, M.

2010-01-01

The design and use of a novel, table-top UV-VIS luminescence spectrometer with two excitation sources is described: a soft X-ray/XUV pulse excitation from the laser-produced plasma in gas puff target of about 4 ns duration, and a conventional N 2 pulse laser excitation at 337 nm (or any other UV-VIS pulse laser excitation). The XUV plasma source generates photons of either quasi-monochromatic (N target, E = 430 eV) or wide (Ar target, E = 200 ∼ 600 eV) spectral range. A combination of both X-ray/XUV and UV-VIS excitation in one experimental apparatus allows to perform comparative luminescence spectra and kinetics measurements under the same experimental conditions. In order to demonstrate the spectrometer, the UV-VIS luminescence spectra and decay kinetics of cerium doped Lu 3 Al 5 O 12 single crystal (LuAG:Ce) scintillator excited by XUV and UV radiation were acquired. Luminescence of doped Ce 3+ ions was studied under XUV 430 eV excitation from the laser-produced nitrogen plasma, and compared with the luminescence under 337 nm (3,68 eV) UV excitation from nitrogen laser. In the former case the excitation energy is deposited in the LuAG host, while in the latter the 4f-5d transition of Ce 3+ is directly excited. Furthermore, LuAG:Ce single crystals and single crystalline films luminescence decay profiles are compared and discussed. (authors)

Synchronization of x-ray pulses to the pump laser in an ultrafast x-ray facility

International Nuclear Information System (INIS)

Corlett, J.N.; Barry, W.; Byrd, J.M.; Schoenlein, R.; Zholents, A.

2002-01-01

Accurate timing of ultrafast x-ray probe pulses emitted from a synchrotron radiation source with respect to a pump laser exciting processes in the sample under study is critical for the investigation of structural dynamics in the femtosecond regime. We describe a scheme for synchronizing femtosecond x-ray pulses relative to a pump laser. X-ray pulses of <100 fs duration are generated from a proposed source based on a recirculating superconducting linac [1,2,3]. Short x-ray pulses are obtained by a process of electron pulse compression, followed by transverse temporal correlation of the electrons, and ultimately x-ray pulse compression. Timing of the arrival of the x-ray pulse with respect to the pump laser is found to be dominated by the operation of the deflecting cavities which provide the transverse temporal correlation of the electrons. The deflecting cavities are driven from a highly stable RF signal derived from a modelocked laser oscillator which is also the origin of the pump l aser pulses

Development of a homogeneous pulse shape discriminating flow-cell radiation detection system

International Nuclear Information System (INIS)

Hastie, K.H.; DeVol, T.A.; Fjeld, R.A.

1999-01-01

A homogeneous flow-cell radiation detection system which utilizes coincidence counting and pulse shape discrimination circuitry was assembled and tested with five commercially available liquid scintillation cocktails. Two of the cocktails, Ultima Flo (Packard) and Mono Flow 5 (National Diagnostics) have low viscosities and are intended for flow applications; and three of the cocktails, Optiphase HiSafe 3 (Wallac), Ultima Gold AB (Packard), and Ready Safe (Beckman), have higher viscosities and are intended for static applications. The low viscosity cocktails were modified with 1-methylnaphthalene to increase their capability for alpha/beta pulse shape discrimination. The sample loading and pulse shape discriminator setting were optimized to give the lowest minimum detectable concentration for methylnaphthalenein a 30 s count time. Of the higher viscosity cocktails, Optiphase HiSafe 3 had the lowest minimum detectable activities for alpha and beta radiation, 0.2 and 0.4 Bq/ml for 233 U and 90 Sr/ 90 Y, respectively, for a 30 s count time. The sample loading was 70% and the corresponding alpha/beta spillover was 5.5%. Of the low viscosity cocktails, Mono Flow 5 modified with 2.5% (by volume) 1-methylnaphthalene resulted in the lowest minimum detectable activities for alpha and beta radiation; 0.3 and 0.5 Bq/ml for 233 U and 90 Sr/ 90 Y, respectively, for a 30 s count time. The sample loading was 50%, and the corresponding alpha/beta spillover was 16.6%. HiSafe 3 at a 10% sample loading was used to evaluate the system under simulated flow conditions

The capability of pulsed laser radiation for cutting band saws hardening

Directory of Open Access Journals (Sweden)

Marinin Evgeny

2017-01-01

Full Text Available The article deals with the possibilities of pulsed laser radiation for hardening the band saws. The regimes of pulsed laser hardening the band saws of 1 mm thick made of tool steel 9CrV are grounded theoretically and experimentally tested. Selected and justified modes of treatment harden in the autohardening mode without additional heat removal. The results of the experimental research of microhardness are presented and formed as a result of processing of the microstructure. Selected modes increase the microhardness of the surface to 8500 MPa and form ultra highly dispersed structure in the surface layer characterized by high resistance to abrasion.

Use of spectra from foil-excited heavy-ion beams to interpret radiation from plasmas

International Nuclear Information System (INIS)

Johnson, B.M.

1978-01-01

Spectra from foil-excited heavy ion beams can be used to investigate the relative abundance and charge state composition of heavy metal contaminants which cause severe radiative energy losses in tokamak-produced plasmas. The degree of ionization of these metals in the tokamak plasma is not well known because of uncertainties in ionization and recombination rates and particle confinement times. Only a few stages of ionization are typically prominent in foil-excited spectra, however, and both the most probable charge state and distribution width are well known. Highly ionized heavy ions (e.g., Ti, Mo, W and Au) which span the range of charge states found in present tokamaks were produced by passing beams from the Brookhaven MP tandem Van de Graaff accelerator facility through 20 μg/cm 2 carbon stripping foils. EUV radiation was recorded with a grazing incidence spectrometer. Comparisons of the beam-foil spectra with radiation from plasmas, and recent direct determinations of atomic oscillator strengths for principal resonance lines of such highly ionized species as Li-like iron (Fe 23+ ), Na-like bromine (Br 24+ ), and Cu-like iodine (I 24+ ) are discussed

Photoionization pathways and thresholds in generation of Lyman-α radiation by resonant four-wave mixing in Kr-Ar mixture

OpenAIRE

Oleg A. Louchev; Norihito Saito; Yu Oishi; Koji Miyazaki; Kotaro Okamura; Jumpei Nakamura; Masahiko Iwasaki; Satoshi Wada

2016-01-01

We develop a set of analytical approximations for the estimation of the combined effect of various photoionization processes involved in the resonant four-wave mixing generation of ns pulsed Lyman-α (L-α) radiation by using 212.556 nm and 820-845 nm laser radiation pulses in Kr-Ar mixture: (i) multi-photon ionization, (ii) step-wise (2+1)-photon ionization via the resonant 2-photon excitation of Kr followed by 1-photon ionization and (iii) laser-induced avalanche ionization produced by genera...

Sensitive detection of chlorine in iron oxide by single pulse and dual pulse laser-induced breakdown spectroscopy

Science.gov (United States)

Pedarnig, J. D.; Haslinger, M. J.; Bodea, M. A.; Huber, N.; Wolfmeir, H.; Heitz, J.

2014-11-01

The halogen chlorine is hard to detect in laser-induced breakdown spectroscopy (LIBS) mainly due to its high excited state energies of 9.2 and 10.4 eV for the most intense emission lines at 134.72 nm and 837.59 nm, respectively. We report on sensitive detection of Cl in industrial iron oxide Fe2O3 powder by single-pulse (SP) and dual-pulse (DP) LIBS measurements in the near infrared range in air. In compacted powder measured by SP excitation (Nd:YAG laser, 532 nm) Cl was detected with limit of detection LOD = 440 ppm and limit of quantitation LOQ = 720 ppm. Orthogonal DP LIBS was studied on pressed Fe2O3 pellets and Fe3O4 ceramics. The transmission of laser-induced plasma for orthogonal Nd:YAG 1064 nm and ArF 193 nm laser pulses showed a significant dependence on interpulse delay time (ipd) and laser wavelength (λL). The UV pulses (λL = 193 nm) were moderately absorbed in the plasma and the Cl I emission line intensity was enhanced while IR pulses (λL = 1064 nm) were not absorbed and Cl signals were not enhanced at ipd = 3 μs. The UV laser enhancement of Cl signals is attributed to the much higher signal/background ratio for orthogonal DP excitation compared to SP excitation and to the increased plasma temperature and electron number density. This enabled measurement at a very short delay time of td ≥ 0.1 μs with respect to the re-excitation pulse and detection of the very rapidly decaying Cl emission with higher efficiency.

EXCITATION TEMPERATURE OF THE WARM NEUTRAL MEDIUM AS A NEW PROBE OF THE Lyα RADIATION FIELD

Energy Technology Data Exchange (ETDEWEB)

Murray, Claire E.; Lindner, Robert R.; Stanimirović, Snežana; Pingel, Nickolas M.; Lawrence, Allen; Babler, Brian L. [Department of Astronomy, University of Wisconsin, Madison, WI 53706 (United States); Goss, W. M.; Jencson, Jacob [National Radio Astronomy Observatory, P.O. Box O, 1003 Lopezville, Socorro, NM 87801 (United States); Heiles, Carl [Radio Astronomy Laboratory, UC Berkeley, 601 Campbell Hall, Berkeley, CA 94720 (United States); Dickey, John [University of Tasmania, School of Maths and Physics, Private Bag 37, Hobart, TAS 7001 (Australia); Hennebelle, Patrick, E-mail: cmurray@astro.wisc.edu [Laboratoire AIM, Paris-Saclay, CEA/IRFU/SAp—CNRS—Université Paris Diderot, F-91191 Gif-sur-Yvette Cedex (France)

2014-02-01

We use the Karl G. Jansky Very Large Array to conduct a high-sensitivity survey of neutral hydrogen (H I) absorption in the Milky Way. In combination with corresponding H I emission spectra obtained mostly with the Arecibo Observatory, we detect a widespread warm neutral medium component with excitation temperature 〈T{sub s}〉=7200{sub −1200}{sup +1800} K (68% confidence). This temperature lies above theoretical predictions based on collisional excitation alone, implying that Lyα scattering, the most probable additional source of excitation, is more important in the interstellar medium (ISM) than previously assumed. Our results demonstrate that H I absorption can be used to constrain the Lyα radiation field, a critical quantity for studying the energy balance in the ISM and intergalactic medium yet notoriously difficult to model because of its complicated radiative transfer, in and around galaxies nearby and at high redshift.

Excited meson radiative transitions from lattice QCD using variationally optimized operators

Energy Technology Data Exchange (ETDEWEB)

Shultz, Christian J. [Old Dominion Univ., Norfolk, VA (United States); Dudek, Jozef J. [Thomas Jefferson National Accelerator Facility (TJNAF), Newport News, VA (United States); Old Dominion Univ., Norfolk, VA (United States); Edwards, Robert G. [Thomas Jefferson National Accelerator Facility (TJNAF), Newport News, VA (United States)

2015-06-02

We explore the use of 'optimized' operators, designed to interpolate only a single meson eigenstate, in three-point correlation functions with a vector-current insertion. These operators are constructed as linear combinations in a large basis of meson interpolating fields using a variational analysis of matrices of two-point correlation functions. After performing such a determination at both zero and non-zero momentum, we compute three-point functions and are able to study radiative transition matrix elements featuring excited state mesons. The required two- and three-point correlation functions are efficiently computed using the distillation framework in which there is a factorization between quark propagation and operator construction, allowing for a large number of meson operators of definite momentum to be considered. We illustrate the method with a calculation using anisotopic lattices having three flavors of dynamical quark all tuned to the physical strange quark mass, considering form-factors and transitions of pseudoscalar and vector meson excitations. In conclusion, the dependence on photon virtuality for a number of form-factors and transitions is extracted and some discussion of excited-state phenomenology is presented.

[Pulse-modulated Electromagnetic Radiation of Extremely High Frequencies Protects Cellular DNA against Damaging Effect of Physico-Chemical Factors in vitro].

Science.gov (United States)

Gapeyev, A B; Lukyanova, N A

2015-01-01

Using a comet assay technique, we investigated protective effects of. extremely high frequency electromagnetic radiation in combination with the damaging effect of X-ray irradiation, the effect of damaging agents hydrogen peroxide and methyl methanesulfonate on DNA in mouse whole blood leukocytes. It was shown that the preliminary exposure of the cells to low intensity pulse-modulated electromagnetic radiation (42.2 GHz, 0.1 mW/cm2, 20-min exposure, modulation frequencies of 1 and 16 Hz) caused protective effects decreasing the DNA damage by 20-45%. The efficacy of pulse-modulated electromagnetic radiation depended on the type of genotoxic agent and increased in a row methyl methanesulfonate--X-rays--hydrogen peroxide. Continuous electromagnetic radiation was ineffective. The mechanisms of protective effects may be connected with an induction of the adaptive response by nanomolar concentrations of reactive oxygen species formed by pulse-modulated electromagnetic radiation.

Speckle Reduction for Ultrasonic Imaging Using Frequency Compounding and Despeckling Filters along with Coded Excitation and Pulse Compression

Directory of Open Access Journals (Sweden)

Joshua S. Ullom

2012-01-01

Full Text Available A method for improving the contrast-to-noise ratio (CNR while maintaining the −6 dB axial resolution of ultrasonic B-mode images is proposed. The technique proposed is known as eREC-FC, which enhances a recently developed REC-FC technique. REC-FC is a combination of the coded excitation technique known as resolution enhancement compression (REC and the speckle-reduction technique frequency compounding (FC. In REC-FC, image CNR is improved but at the expense of a reduction in axial resolution. However, by compounding various REC-FC images made from various subband widths, the tradeoff between axial resolution and CNR enhancement can be extended. Further improvements in CNR can be obtained by applying postprocessing despeckling filters to the eREC-FC B-mode images. The despeckling filters evaluated were the following: median, Lee, homogeneous mask area, geometric, and speckle-reducing anisotropic diffusion (SRAD. Simulations and experimental measurements were conducted with a single-element transducer (f/2.66 having a center frequency of 2.25 MHz and a −3 dB bandwidth of 50%. In simulations and experiments, the eREC-FC technique resulted in the same axial resolution that would be typically observed with conventional excitation with a pulse. Moreover, increases in CNR of 348% were obtained in experiments when comparing eREC-FC with a Lee filter to conventional pulsing methods.

Study of performance of electronic dosemeters in continuous and pulsed X-radiation beams

International Nuclear Information System (INIS)

Guimaraes, Margarete Cristina

2014-01-01

Personal radiation monitoring is a basic procedure to verify the compliance to regulatory requirements for radiological protection. Electronic personal dosimeters (EPD) based on solid state detectors have largely been used for personnel monitoring; including for pulsed radiation beams where their responses are not well known and deficiencies have been reported. In this work, irradiation conditions for testing the response of EPDs in both continuous and pulsed X-ray beams were studied to be established in a constant potential Seifert-Pantak and in a medical Pulsar 800 Plus VMI X-ray machines. Characterization of X-ray beams was done in terms of tube voltage, half-value layer, mean energy and air kerma rate. A Xi R/F Unfors solid state dosimeter used as reference for air kerma measurements was verified against a RC-6 and 10X6-6 Radical ionization chambers as far its metrological coherence. Rad-60 RADOS, PDM- 11 Aloka and EPD MK2 Thermo electron EPDs were selected to be tested in terms of relative intrinsic error and energy response in similar to IEC RQR, IEC RQA and ISO N reference radiations. Results demonstrated the reliability of the solid state Xi R/F Unfors dosimeter to be as reference dosimeter although its response was affected by heavily filtered beams. Results also showed that relative intrinsic errors in the response of the EPDs in terms of personal dose equivalent, Hp(10), were higher than the requirement established for continuous beams. In pulsed beams, some EPDs showed inadequate response and high relative intrinsic errors. This work stressed the need of performing additional checks for EPDs, besides the limited 137 Cs beam calibration, before using them in pulsed X-ray beams. (author)

Nonlinear behavior of photoluminescence from silicon particles under two-photon excitation

International Nuclear Information System (INIS)

Xu Xingsheng; Yokoyama, Shiyoshi

2011-01-01

Two-photon excited fluorescence (TPEF) under continuous-wave excitation from silicon particles produced by a pulsed laser is investigated. Spectra and images of TPEF from silicon particles are studied under different excitation intensities and operation modes (continuous wave or pulse). It is found that the photoluminescence depends superlinearly on the excitation intensity and that the spectral shape and peaks vary with different silicon particles. The above phenomena show the nonlinear behavior of TPEF from silicon particles, and stimulated emission is a possible process.

Technical specifications manual for the MARK-1 pulsed ionizing radiation detection system

International Nuclear Information System (INIS)

Lawrence, R.S.; Harker, Y.D.; Jones, J.L.; Hoggan, J.M.

1993-03-01

The MARK-1 detection system was developed by the Idaho National Engineering Laboratory for the US Department of Energy Office of Arms Control and Nonproliferation. The completely portable system was designed for the detection and analysis of intense photon emissions from pulsed ionizing radiation sources. This manual presents the technical design specifications for the MARK-1 detection system and was written primarily to assist the support or service technician in the service, calibration, and repair of the system. The manual presents the general detection system theory, the MARK-1 component design specifications, the acquisition and control software, the data processing sequence, and the system calibration procedure. A second manual entitled: Volume 2: Operations Manual for the MARK-1 Pulsed Ionizing Radiation Detection System (USDOE Report WINCO-1108, September 1992) provides a general operational description of the MARK-1 detection system. The Operations Manual was written primarily to assist the field operator in system operations and analysis of the data

Control of HOD photodissociation dynamics via bond-selective infrared multiphoton excitation and a femtosecond ultraviolet laser pulse

DEFF Research Database (Denmark)

Amstrup, Bjarne; Henriksen, Niels Engholm

1992-01-01

moment, excites the molecule to a dissociative electronic state. We consider the HOD molecule which is ideal due to the local mode structure of the vibrational states. It is shown that selective and localized bond stretching can be created in simple laser fields. When such a nonstationary vibrating HOD...... molecule is photodissociated with a short laser pulse (~5 fs) complete selectivity between the channels H+OD and D+OH is observed over the entire absorption band covering these channels. The Journal of Chemical Physics is copyrighted by The American Institute of Physics....

The influence of collapse wall on self-excited oscillation pulsed jet nozzle performance

International Nuclear Information System (INIS)

Fang, Z L; Kang, Y; Yang, X F; Yuan, B; Li, D

2012-01-01

The self-excited oscillation pulsed jet (SOPJ) is widely used owing to its simple structure and good separation of pressure source and system. The structure of nozzle is one of the main factors that influence the performance of the SOPJ nozzle. Upper collapse wall and lower collapse wall is important to the formation and transmission of eddy in oscillation cavity. In this paper, the influence of collapse wall on SOPJ nozzle was analyzed by numerical simulation. The LES algorithm was used to simulate the flow of different combinations of collapse wall. The result showed that when both collapse walls are of the same type, the SOPJ nozzle will have a good performance; the influence of upper collapse wall is more obvious than lower one; model of two-semi-circle upper collapse wall is the first choice when we design SOPJ nozzle.

Quasi-real-time photon pulse duration measurement by analysis of FEL radiation spectra

Energy Technology Data Exchange (ETDEWEB)

Engel, Robin, E-mail: robin.engel@uni-oldenburg.de [Deutsches Elektronen-Synchrotron, Notkestrasse 85, D-22603 Hamburg (Germany); Institut für Physik, Carl von Ossietzky Universität Oldenburg, D-26111 Oldenburg (Germany); Institut für Laser und Optik, Hochschule Emden/Leer, University of Applied Sciences, Constantiaplatz 4, D-26723 Emden (Germany); Düsterer, Stefan; Brenner, Günter [Deutsches Elektronen-Synchrotron, Notkestrasse 85, D-22603 Hamburg (Germany); Teubner, Ulrich [Deutsches Elektronen-Synchrotron, Notkestrasse 85, D-22603 Hamburg (Germany); Institut für Physik, Carl von Ossietzky Universität Oldenburg, D-26111 Oldenburg (Germany); Institut für Laser und Optik, Hochschule Emden/Leer, University of Applied Sciences, Constantiaplatz 4, D-26723 Emden (Germany)

2016-01-01

Considering the second-order spectral correlation function of SASE-FEL radiation allows a real-time observation of the photon pulse duration during spectra acquisition. For photon diagnostics at free-electron lasers (FELs), the determination of the photon pulse duration is an important challenge and a complex task. This is especially true for SASE FELs with strongly fluctuating pulse parameters. However, most techniques require an extensive experimental setup, data acquisition and evaluation time, limiting the usability in all-day operation. In contrast, the presented work uses an existing approach based on the analysis of statistical properties of measured SASE FEL spectra and implements it as a software tool, integrated in FLASH’s data acquisition system. This allows the calculation of the average pulse durations from a set of measured spectral distributions with only seconds of delay, whenever high-resolution spectra are recorded.

Dissipation of the electronic excitation energy in fluorides with different type of a crystal lattice

International Nuclear Information System (INIS)

Lisitsyn, V.M.; Grechkina, T. V.; Korepanov, V.I.; Lisitsyna, L.A.

2004-01-01

Full text: In this paper we present results of comparison of efficiency creations of primary defects in crystals of fluorides of two different lattice structures: stone salt - LiF and rutile MgF 2 . We have used the methods with nanosecond time-resolved of pulse spectroscopy and found laws of creation and evolution self-trapped exciton (STE) and the F centers in a temperature range from 12.5 to 500 K and a time interval from 10 -8 to 10 -1 s after the ending of influence of a pulse electron. The density of excitation of crystals in a pulse is no more than 0.1 J·cm -3 , average energy electrons made 200 keV, duration electron pulse - 7 ns. It is established, that in crystal LiF under action of radiation are created STE two types which have various spectral-kinetic parameters absorption and emission transitions, various values of activation energy of processes of a post-industrial relaxation and different character of temperature dependences of creation efficiency under action electron pulse. In the field of low temperatures (12.5 K) created on center STE has absorption bands on 5.5 and 5.1 eV and emission band on 5.8 eV. Off-center STE has absorption on 5.3 and 4.75 eV and emission on 4.4 eV bands and are created in the interval 12.5-170 K with peak efficiency h area 60 K. In crystal MgF 2 at low temperatures (20 K) under action of radiation one STE with a nucleus occupying off-center configuration, having luminescence band on 3.2 eV and a series absorption transitions in area 4-5.5 eV is created. Concurrently with STE in both crystals under action of a pulse electron the F-centers with efficiency, not dependent on temperature of a crystal in area 20-100 K are created. There are two alternative processes under action of an irradiation with growth of temperature higher 100 K: reducing of STE creation and increasing of F centers creation. In both crystals quenching temperature of luminescence STE at T>60 K which is not accompanied by growth of efficiency of creation

Proposals of electronic-vibrational energy relaxation studies by using laser pulses synchronized with IR-SR pulses

International Nuclear Information System (INIS)

Nakagawa, Hideyuki

2000-01-01

Synchrotron radiation is expected to be the sharp infrared light source for the advanced experiments on IR and FIR spectroscopy in wide research fields. Especially, synchronized use of SR with VIS and/or UV laser light is to be a promising technique for the research on the dynamical properties of the photo-excited states in condensed materials. Some proposals are attempted for high resolution IR spectroscopy to elucidate fine interaction of molecular ions in crystalline solids with their environmental field and for time-resolved IR spectroscopic studies on the electronic and vibrational energy relaxation by using laser pulses synchronized with IR-SR pulses. Several experimental results are presented in relevance to the subjects; on high-resolution FTIR spectra of cyanide ions and metal cyanide complexes in cadmium halide crystals, on the energy up-conversion process among the vibrational levels of cyanide ions in alkali halide crystals, and on the electronic-to-vibrational energy conversion process in metal cyanide complexes. (author)

Test of the neoclassical theory of radiation in a weakly excited atomic system

International Nuclear Information System (INIS)

Brink, G.O.

1975-01-01

The neoclassical theory of radiation predicts that the decay rate of an excited atomic state depends on the population density of the lower state. Experimental evidence is presented here which shows that in the case of 39 K the decay rate is in agreement with the predictions of quantum electrodynamics and definitely in disagreement with the neoclassical theory

The Formation of a Power Multi-Pulse Extreme Ultraviolet Radiation in the Pulse Plasma Diode of Low Pressure

Directory of Open Access Journals (Sweden)

Ievgeniia V. Borgun

2013-01-01

Full Text Available In this paper results are presented on experimental studies of the temporal characteristics of spike extreme ultraviolet (EUV radiation in the spectral range of 12.2 ÷ 15.8 nm from the anode region of high-current (I = 40 kA pulsed discharges in tin vapor. It is observed that the intense multi-spike radiation in this range arises at an inductive stage of the discharge. It has been shown that the radiation spikes correlate with the sharp increase of active resistance and of pumped power, due to plasma heating by an electron beam, formed in the double layer of charged particles. It has been observed that for large number of spikes the conversion efficiency of pumped energy into radiationat double layer formation is essentially higher in comparison with collisional heating.

Kharkov 3-GeV pulse stretcher ring as a source of synchrotron radiation

International Nuclear Information System (INIS)

Boldyshev, V.F.; Gladkikh, P.I.; Grigor'ev, Y.N.; Guk, I.S.; Efimov, S.V.; Karnaukhov, I.M.; Kononenko, S.G.; Mocheshnikov, N.I.; Popkov, Y.P.; Tarasenko, A.S.; Telegin, Y.N.; Chechetenko, V.F.; Shcherbakov, A.A.; Titov, V.A.; Nagaenko, M.G.

1989-01-01

The article discusses the possibility of using the pulse stretcher ring, designed at the Kharkov Institute of Physics and Technology, as a synchrotron radiation source (SRS). Comparison is made between our SRS design parameters and those of other dedicated SRSs

CO2 laser pulse shortening by laser ablation of a metal target

International Nuclear Information System (INIS)

Donnelly, T.; Mazoyer, M.; Lynch, A.; O'Sullivan, G.; O'Reilly, F.; Dunne, P.; Cummins, T.

2012-01-01

A repeatable and flexible technique for pulse shortening of laser pulses has been applied to transversely excited atmospheric (TEA) CO 2 laser pulses. The technique involves focusing the laser output onto a highly reflective metal target so that plasma is formed, which then operates as a shutter due to strong laser absorption and scattering. Precise control of the focused laser intensity allows for timing of the shutter so that different temporal portions of the pulse can be reflected from the target surface before plasma formation occurs. This type of shutter enables one to reduce the pulse duration down to ∼2 ns and to remove the low power, long duration tails that are present in TEA CO 2 pulses. The transmitted energy is reduced as the pulse duration is decreased but the reflected power is ∼10 MW for all pulse durations. A simple laser heating model verifies that the pulse shortening depends directly on the plasma formation time, which in turn is dependent on the applied laser intensity. It is envisaged that this plasma shutter will be used as a tool for pulse shaping in the search for laser pulse conditions to optimize conversion efficiency from laser energy to useable extreme ultraviolet (EUV) radiation for EUV source development.

Electronic perturbation investigations into excitation and ionization in the millisecond pulsed glow discharge plasma

International Nuclear Information System (INIS)

Li Lei; Robertson-Honecker, Jennifer; Vaghela, Vishal; King, Fred L.

2006-01-01

This study employed a power perturbation method to examine the energy transfer processes at different locations within the afterpeak regime of a millisecond pulsed glow discharge plasma. Brief power perturbation pulses were applied during the afterpeak regime altering the environment of the collapsing plasma. Responses of several transitions to the power perturbations were measured via atomic emission and absorption spectroscopic methods at various distances from the surface of the cathode. The experimental data provide further insight into the energy transfer processes that occur at different spatial locations and in different temporal regimes of these pulsed glow discharge plasmas. Although the enhancement of the large population of metastable argon atoms is again confirmed, the mechanism responsible for this enhancement remains unclear. The most likely possibility involves some form of ion-electron recombination followed by radiative relaxation of the resulting species. The metastable argon atoms subsequently Penning ionize sputtered copper atoms which then appear to undergo a similar ion-electron recombination process yielding variable degrees of observable afterpeak emission for copper atom transitions. The kinetic information of these processes was approximated from the corresponding relaxation time. The electron thermalization time allowing for recombination with ions was found to be ∼25 μs after the discharge power termination

TH-F-202-03: Advances in MRI for Radiation Therapy

Energy Technology Data Exchange (ETDEWEB)

Cai, J. [Duke University Medical Center (United States)

2016-06-15

MRI has excellent soft tissue contrast and can provide both anatomical and physiological information. It is becoming increasingly important in radiation therapy for treatment planning, image-guided radiation therapy, and treatment assessment. It is critically important at this time point to educate and update our medical physicists about MRI to prepare for the upcoming surge of MRI applications in radiation therapy. This session will review important basics of MR physics, pulse sequence designs, and current radiotherapy application, as well as showcase exciting new developments in MRI that can be potentially useful in radiation therapy. Learning Objectives: To learn basics of MR physics and understand the differences between various pulse sequences To review current applications of MRI in radiation therapy.To discuss recent MRI advances for future MRI guided radiation therapy Partly supported by NIH (1R21CA165384).; W. Miller, Research supported in part by Siemens Healthcare; G. Li, My clinical research is in part supported by NIH U54CA137788. I have a collaborative research project with Philips Healthcare.; J. Cai, jing cai.

TH-F-202-03: Advances in MRI for Radiation Therapy

International Nuclear Information System (INIS)

Cai, J.

2016-01-01

MRI has excellent soft tissue contrast and can provide both anatomical and physiological information. It is becoming increasingly important in radiation therapy for treatment planning, image-guided radiation therapy, and treatment assessment. It is critically important at this time point to educate and update our medical physicists about MRI to prepare for the upcoming surge of MRI applications in radiation therapy. This session will review important basics of MR physics, pulse sequence designs, and current radiotherapy application, as well as showcase exciting new developments in MRI that can be potentially useful in radiation therapy. Learning Objectives: To learn basics of MR physics and understand the differences between various pulse sequences To review current applications of MRI in radiation therapy.To discuss recent MRI advances for future MRI guided radiation therapy Partly supported by NIH (1R21CA165384).; W. Miller, Research supported in part by Siemens Healthcare; G. Li, My clinical research is in part supported by NIH U54CA137788. I have a collaborative research project with Philips Healthcare.; J. Cai, jing cai

Study of the ionization of sodium vapor in the presence of resonant laser radiation

International Nuclear Information System (INIS)

Carre, B.

1986-06-01

Ionization of a diffuse sodium jet, excited by laser radiation (D2 resonance), either continuous or pulsed, is studied by electron spectroscopy. Results show: associative ionization (AI) in the collision of two Na(3p) excited atoms; occupancy of highly excited nl states in energy association collisions of two Na(3p) followed by Penning collisional ionization (CI) in the system Na(nl) + Na(3p); heating of electrons by 1, 2, or 3 superelastic collisions with Na(3p). For both the excitation cases (continuous or pulsed source) analysis of experiment results leads to a description of the whole of the ionized medium, characterized as being low density and the site of the ambipolar diffusion of charged particles. A highly simplified model describes the kinetic and electrokinetic equilibrium (continuous case) in which the different populations of distinct nonthermalized energy (low energy primary electrons, hot electrons) play specific roles. The cross sections associated with AI and CI are estimated from experiment results using the model [fr

Comparison of ATLOG and Xyce for Bell Labs Electromagnetic Pulse Excitation of Finite-Long Dissipative Conductors over a Ground Plane.

Energy Technology Data Exchange (ETDEWEB)

campione, Salvatore [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Warne, Larry K. [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Schiek, Richard [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Basilio, Lorena I. [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

2017-09-01

This report details the modeling results for the response of a finite-length dissipative conductor interacting with a conducting ground to the Bell Labs electromagnetic pulse excitation. We use both a frequency-domain and a time-domain method based on transmission line theory through a code we call ATLOG - Analytic Transmission Line Over Ground. Results are compared to the circuit simulator Xyce for selected cases. Intentionally Left Blank

Transient pulse analysis of ionized electronics exposed to γ-radiation generated from a relativistic electron beam

Science.gov (United States)

Min, Sun-Hong; Kwon, Ohjoon; Sattorov, Matlabjon; Baek, In-Keun; Kim, Seontae; Hong, Dongpyo; Jeong, Jin-Young; Jang, Jungmin; Bera, Anirban; Barik, Ranjan Kumar; Bhattacharya, Ranajoy; Cho, Ilsung; Kim, Byungsu; Park, Chawon; Jung, Wongyun; Park, Seunghyuk; Park, Gun-Sik

2018-02-01

When a semiconductor element is irradiated with radiation in the form of a transient pulse emitted from a nuclear explosion, a large amount of charge is generated in a short time in the device. A photocurrent amplified in a certain direction by these types of charges cause the device to break down and malfunction or in extreme cases causes them to burn out. In this study, a pulse-type γ-ray generator based on a relativistic electron beam accelerator (γ=2.2, β=0.89) which functions by means of tungsten impingement was constructed and tested in an effort to investigate the process and effects of the photocurrent formed by electron hole pairs (EHP) generated in a pMOSFET device when a transient radiation pulse is incident in the device. The pulse-type γ-ray irradiating device used here to generate the electron beam current in a short time was devised to allow an increase in the irradiation dose. A precise signal processing circuit was constructed to measure the photocurrent of the small signal generated by the pMOSFET due to the electron beam accelerator pulse signal from the large noise stemming from the electromagnetic field around the relativistic electron beam accelerator. The pulse-type γ-ray generator was installed to meet the requirements of relativistic electron beam accelerators, and beam irradiation was conducted after a beam commissioning step.

Off-resonant vibrational excitation: Orientational dependence and spatial control of photofragments

DEFF Research Database (Denmark)

Machholm, Mette; Henriksen, Niels Engholm

2000-01-01

Off-resonant and resonant vibrational excitation with short intense infrared (IR) laser pulses creates localized oscillating wave packets, but differs by the efficiency of the excitation and surprisingly by the orientational dependence. Orientational selectivity of the vibrational excitation...... of randomly oriented heteronuclear diatomic molecules can be obtained under simultaneous irradiation by a resonant and an off-resonant intense IR laser pulse: Molecules with one initial orientation will be vibrationally excited, while those with the opposite orientation will be at rest. The orientation-dependent...... distribution. (C) 2000 American Institute of Physics....

Development and performance test of picosecond pulse x-ray excited streak camera system for scintillator characterization

International Nuclear Information System (INIS)

Yanagida, Takayuki; Fujimoto, Yutaka; Yoshikawa, Akira

2010-01-01

To observe time and wavelength-resolved scintillation events, picosecond pulse X-ray excited streak camera system is developed. The wavelength range spreads from vacuum ultraviolet (VUV) to near infrared region (110-900 nm) and the instrumental response function is around 80 ps. This work describes the principle of the newly developed instrument and the first performance test using BaF 2 single crystal scintillator. Core valence luminescence of BaF 2 peaking around 190 and 220 nm is clearly detected by our system, and the decay time turned out to be of 0.7 ns. These results are consistent with literature and confirm that our system properly works. (author)

Biological effectiveness of pulsed and continuous neutron radiation for cells of yeast Saccharomyces

International Nuclear Information System (INIS)

Tsyb, T.S.; Komarova, E.V.; Potetnya, V.I.; Obaturov, G.M.

2001-01-01

Data are presented on biological effectiveness of fast neutrons generated by BR-10 reactor (dose rate up to 3.8 Gy/s) in comparison with neutrons of pulsed BARS-6 reactor (dose rate ∼6x10 6 Gy/s) for yeast Saccharomyces vini cells of a wild type Menri 139-B and radiosensitive Saccharomyces cerevisiae (rad52/rad52; rad54/rad54) mutants which are defective over different systems of DNA reparation. Value of relative biological efficiency (RBE) of continuous radiation for wild stam is from 3.5 up to 2.5 when survival level being 75-10 %, and RBE of pulsed neutron radiation is in the limits of 2.0-1.7 at the same levels. For mutant stam the value of RBE (1.4-1.6) of neutrons is constant at all survival levels and does not depend on dose rate [ru

Magnetic field effects on ultrafast lattice compression dynamics of Si(111) crystal when excited by linearly-polarized femtosecond laser pulses

Science.gov (United States)

Hatanaka, Koji; Odaka, Hideho; Ono, Kimitoshi; Fukumura, Hiroshi

2007-03-01

Time-resolved X-ray diffraction measurements of Si (111) single crystal are performed when excited by linearly-polarized femtosecond laser pulses (780 nm, 260 fs, negatively-chirped, 1 kHz) under a magnetic field (0.47 T). Laser fluence on the sample surface is 40 mJ/cm^2, which is enough lower than the ablation threshold at 200 mJ/cm^2. Probing X-ray pulses of iron characteristic X-ray lines at 0.193604 and 0.193998 nm are generated by focusing femtosecond laser pulses onto audio-cassette tapes in air. Linearly-polarized femtosecond laser pulse irradiation onto Si(111) crystal surface induces transient lattice compression in the picosecond time range, which is confirmed by transient angle shift of X-ray diffraction to higher angles. Little difference of compression dynamics is observed when the laser polarization is changed from p to s-pol. without a magnetic field. On the other hand, under a magnetic field, the lattice compression dynamics changes when the laser is p-polarized which is vertical to the magnetic field vector. These results may be assigned to photo-carrier formation and energy-band distortion.

Comparison of high-voltage ac and pulsed operation of a surface dielectric barrier discharge

Science.gov (United States)

Williamson, James M.; Trump, Darryl D.; Bletzinger, Peter; Ganguly, Biswa N.

2006-10-01

A surface dielectric barrier discharge (DBD) in atmospheric pressure air was excited either by low frequency (0.3-2 kHz) high-voltage ac or by short, high-voltage pulses at repetition rates from 50 to 600 pulses s-1. The short-pulse excited discharge was more diffuse and did not have the pronounced bright multiple cathode spots observed in the ac excited discharge. The discharge voltage, current and average power deposited into the discharge were calculated for both types of excitation. As a measure of plasma-chemical efficiency, the ozone number density was measured by UV absorption as a function of average deposited power. The density of ozone produced by ac excitation did not increase so rapidly as that produced by short-pulse excitation as a function of average power, with a maximum measured density of ~3 × 1015 cm-3 at 25 W. The maximum ozone production achieved by short-pulse excitation was ~8.5 × 1015 cm-3 at 20 W, which was four times greater than that achieved by ac excitation at the same power level.

High-density optical data storage based on grey level recording in photobleaching polymers using two-photon excitation under ultrashort pulse and continuous wave illumination

International Nuclear Information System (INIS)

Ganic, D.; Day, D.; Gu, M.

1999-01-01

Full text: Two-photon excitation has been employed in three-dimensional optical data storage by many researchers in an attempt to increase the storage density of a given material. The probability of two-photon excitation is proportional to the squared intensity of the incident light; this effect produces excitation only within a small region of the focus spot. Another advantage of two-photon excitation is the use of infrared illumination, which results in the reduction of scattering and enables the recording of layers at a deep depth in a thick material. The storage density thus obtained using multi-layered bit optical recording can be as high as Tbit/cm 3 . To increase this storage density even further, grey level recording can be employed. This method utilises variable exposure times of a laser beam focused into a photobleaching sample. As a result, the bleached area possesses a certain pixel value which depends upon the exposure time; this can increase the storage density many times depending upon the number of grey levels used. Our experiment shows that it is possible to attain grey level recording using both ultrashort pulsed and continuous-wave illumination. Although continuous wave illumination requires an average power of approximately 2 orders of magnitude higher than that for ultrashort pulsed illumination, it is a preferred method of recording due to its relatively low system cost and compactness. Copyright (1999) Australian Optical Society

Dispersive shock mediated resonant radiations in defocused nonlinear medium

Science.gov (United States)

Bose, Surajit; Chattopadhyay, Rik; Bhadra, Shyamal Kumar

2018-04-01

We report the evolution of resonant radiation (RR) in a self-defocused nonlinear medium with two zero dispersion wavelengths. RR is generated from dispersive shock wave (DSW) front when the pump pulse is in non-solitonic regime close to first zero dispersion wavelength (ZDW). DSW is responsible for pulse splitting resulting in the generation of blue solitons when leading edge of the pump pulse hits the first ZDW. DSW also generates a red shifted dispersive wave (DW) in the presence of higher order dispersion coefficients. Further, DSW through cross-phase modulation with red shifted dispersive wave (DW) excites a localized radiation. The presence of zero nonlinearity point in the system restricts red-shift of RR and enhances the red shifting of DW. It also helps in the formation of DSW at shorter distance and squeezes the solitonic region beyond second zero dispersion point. Predicted results indicate that the spectral evolution depends on the product of Kerr nonlinearity and group velocity dispersion.

Laser excitation of the n=3 level of positronium for antihydrogen production

CERN Document Server

Aghion, S; Ariga, A; Ariga, T; Bonomi, G; Braunig, P; Bremer, J; Brusa, R S; Cabaret, L; Caccia, M; Caravita, R; Castelli, F; Cerchiari, G; Chlouba, K; Cialdi, S; Comparat, D; Consolati, G; Demetrio, A; Di Noto, L; Doser, M; Dudarev, A; Ereditato, A; Evans, C; Ferragut, R; Fesel, J; Fontana, A; Forslund, O K; Gerber, S; Giammarchi, M; Gligorova, A; Gninenko, S N; Guatieri, F; Haider, S; Holmestad, H; Huse, T; Jernelv, I L; Jordan, E; Kellerbauer, A; Kimura, M; Koetting, T; Krasnicky, D; Lagomarsino, V; Lansonneur, P; Lebrun, P; Lehner, S; Liberadzka, J; Malbrunot, C; Mariazzi, S; Marx, L; Matveev, V A; Mazzotta, Z; Nebbia, G; Nedelec, P; Oberthaler, M K; Pacifico, N; Pagano, D; Penasa, L; Petracek, V; Pistillo, C; Prelz, F; Prevedelli, M; Ravelli, L; Resch, L; Rienacker, B; Røhne, O M; Rotondi, A; Sacerdoti, M; Sandaker, H; Santoro, R; Scampoli, P; Smestad, L; Sorrentino, F; Spacek, M; Storey, J; Strojek, I M; Testera, G; Tietje, I; Vamosi, S; Widmann, E; Yzombard, P; Zmeskal, J; Zurlo, N.

2016-01-01

We demonstrate laser excitation of the n=3 state of positronium (Ps) in vacuum. A specially designed high-efficiency pulsed slow positron beam and single shot positronium annihilation lifetime spectroscopy were used to produce and detect Ps. Pulsed laser excitation of n=3 level at 205 nm was monitored via Ps photoionization induced by a second intense laser pulse at 1064 nm. About 15% of the overall positronium emitted in vacuum was excited to n=3 and photoionized. Saturation of both the n=3 excitation and the following photoionization was observed and is explained by a simple rate equation model. Scanning the laser frequency allowed us to extract the positronium transverse temperature related to the width of the Doppler-broadened line. Moreover, preliminary observation of excitation to Rydberg states (n = 15...17) using n=3 as intermediate level was observed, giving an independent confirmation of efficient excitation to the 33P state.

Simulation of continious radiation effect on semiconductors by the pulse irradiation

International Nuclear Information System (INIS)

Radyuk, I.A.; Fejgin, O.O.; Shein, O.V.

1986-01-01

The problem of the laboratory radiation modelling of semiconductor devices and integrated circuits has been under consideration. The condition of adequacy of influencing the pulsed and continuous irradiation semiconductor devices and integrated circuits have been established. The methods of comparing and calculating the influences have been discussed. A number of expressions describing the connection between the parameters of impulced and continuous irradiation have been considered

Dynamics of photoprocesses induced by femtosecond infrared radiation in free molecules and clusters of iron pentacarbonyl

International Nuclear Information System (INIS)

Kompanets, V. O.; Lokhman, V. N.; Poydashev, D. G.; Chekalin, S. V.; Ryabov, E. A.

2016-01-01

The dynamics of photoprocesses induced by femtosecond infrared radiation in free Fe(CO) 5 molecules and their clusters owing to the resonant excitation of vibrations of CO bonds in the 5-μm range has been studied. The technique of infrared excitation and photoionization probing (λ = 400 nm) by femtosecond pulses has been used in combination with time-of-flight mass spectrometry. It has been found that an infrared pulse selectively excites vibrations of CO bonds in free molecules, which results in a decrease in the yield of the Fe(CO) 5 + molecular ion. Subsequent relaxation processes have been analyzed and the results have been interpreted. The time of the energy transfer from excited vibrations to other vibrations of the molecule owing to intramolecular relaxation has been measured. The dynamics of dissociation of [Fe(CO) 5 ] n clusters irradiated by femtosecond infrared radiation has been studied. The time dependence of the yield of free molecules has been measured under different infrared laser excitation conditions. We have proposed a model that well describes the results of the experiment and makes it possible, in particular, to calculate the profile of variation of the temperature of clusters within the “evaporation ensemble” concept. The intramolecular and intracluster vibrational relaxation rates in [Fe(CO) 5 ] n clusters have been estimated.

Infrared response of YBa2Cu3O7-δ films to pulsed, broadband synchrotron radiation

International Nuclear Information System (INIS)

Carr, G.L.; Quijada, M.; Tanner, D.B.; Etemad, S.; DeRosa, F.; Venkatesan, T.; Dutta, B.; Hemmick, D.; Xi, X.

1990-01-01

We report studies of a thin high T c film operating as a fast bolometric detector of infrared radiation. The film has a response of infrared radiation. The film has a response of several mV when exposed to a 1 W, 1 ns duration broadband infrared pulse. The decay after the pulse was about 4 ns. The temperature dependence of the response accurately tracked dR/dT. A thermal model, in which the film's temperature varies relative to the substrate, provides a good description of the response. We find no evidence for other (non-bolometric) response mechanisms for temperatures near or well below T c . 13 refs., 4 figs

Dynamic View on Nanostructures: A Technique for Time Resolved Optical Luminescence Using Synchrotron Light Pulses at SRC, APS, and CLS

International Nuclear Information System (INIS)

Heigl, F.; Jurgensen, A.; Zhou, X.-T.; Lam, S.; Murphy, M.; Ko, J.Y.P.; Sham, T.K.; Rosenberg, R.A.; Gordon, R.; Brewe, D.; Regier, T.; Armelao, L.

2007-01-01

We present an experimental technique using the time structure of synchrotron radiation to study time resolved X-ray excited optical luminescence. In particular we are taking advantage of the bunched distribution of electrons in a synchrotron storage ring, giving short x-ray pulses (10-10 2 picoseconds) which are separated by non-radiating gaps on the nano- to tens of nanosecond scale - sufficiently wide to study a broad range of optical decay channels observed in advanced nanostructured materials.

Radiative charge-transfer lifetime of the excited state of (NaCa)+

International Nuclear Information System (INIS)

Makarov, Oleg P.; Cote, R.; Michels, H.; Smith, W.W.

2003-01-01

New experiments were proposed recently to investigate the regime of cold atomic and molecular ion-atom collision processes in a special hybrid neutral-atom-ion trap under high-vacuum conditions. We study the collisional cooling of laser precooled Ca + ions by ultracold Na atoms. Modeling this process requires knowledge of the radiative lifetime of the excited singlet A 1 Σ + state of the (NaCa) + molecular system. We calculate the rate coefficient for radiative charge transfer using a semiclassical approach. The dipole radial matrix elements between the ground and the excited states, and the potential curves were calculated using complete active space self-consistent field and Moeller-Plesset second-order perturbation theory with an extended Gaussian basis, 6-311+G (3df). The semiclassical charge-transfer rate coefficient was averaged over a thermal Maxwellian distribution. In addition, we also present elastic collision cross sections and the spin-exchange cross section. The rate coefficient for charge transfer was found to be 2.3x10 -16 cm 3 /sec, while those for the elastic and spin-exchange cross sections were found to be several orders of magnitude higher (1.1x10 -8 cm 3 /sec and 2.3x10 -9 cm 3 /sec, respectively). This confirms our assumption that the milli-Kelvin regime of collisional cooling of calcium ions by sodium atoms is favorable with the respect to low loss of calcium ions due to the charge transfer

Study on pulsed radiation generation in the accelerator AKVAGEN; Issledovanie po generatsii impul`sa izlucheniya uskoritelya AKVAGEN

Energy Technology Data Exchange (ETDEWEB)

Bakulin, Yu P [and others

1994-12-31

The pulse accelerator AKVAGEN is created according to a circuit of as single forming line, charged from two pulse transformers up to 1.5 voltage. Typical irradiation levels are presented. The accelerator x radiation efficiency calculated makes up for Si and SiC, SiO{sub 2}, GaAs compounds.

Compression and radiation of high-power short rf pulses. II. A novel antenna array design with combined compressor/radiator elements

KAUST Repository

Sirenko, Kostyantyn; Pazynin, Vadim L.; Sirenko, Yu K.; Bagci, Hakan

2011-01-01

The paper discusses the radiation of compressed high power short RF pulses using two different types of antennas: (i) A simple monopole antenna and (ii) a novel array design, where each of the elements is constructed by combining a compressor and a

Wave-packet dynamics in alkaline dimers. Investigation and control through coherent excitation with fs-pulses; Wellenpaketdynamik in Alkali-Dimeren. Untersuchung und Steuerung durch kohaerente Anregung mit fs-Pulsen

Energy Technology Data Exchange (ETDEWEB)

Sauer, F.N.B.

2007-07-01

During my PhD thesis I investigated alkaline dimers with coherent control in a molecular beam as well as with pump-probe spectroscopy in a magneto-optical trap (MOT). The aim of the coherent control experiments were the isotope selective ionization with phase- and amplitude-shaped fs-pulses. Chapter 4 described the gained results of isotope selective ionization of NaK and KRb in a molecular beam by using different pulse formers. For the NaK dimer was the reached optimization factor R{sub Ph} and {sub Ampl}{sup 770}=R{sub max}/R{sub min}=25 between maximization and minimization of the isotopomer ratio ({sup 23}Na{sup 39}K){sup +}/({sup 23}Na{sup 41}K){sup +} with phase and amplitude modulation of the fs-pulse with a central wavelength of {lambda}=770 nm. From the electronic ground-state X(1){sup 1}{sigma}{sup +};{nu}''=0 transfers a one-photon-excitation population in the first excited A(2) {sup 1}{sigma}{sup +} state. The coherent control experiment on KRb was used to maximize and minimize the isotopomer ratio ({sup 124}KRb){sup +}/({sup 126}KRb){sup +}. It was the first coherent control experiment with a spectral resolution of 1.84 cm{sup -1}/Pixel. For the phase and amplitude optimization was the received optimization factor between minimization and maximization of the isotopomer ratio R{sub Ph} and {sub Ampl}=R{sub max}/R{sub min}=7 at a central wavelength of 840 nm. The results showed a stepwise excitation process from the electronic ground-state in the first excited (2){sup 1}{sigma}{sup +} state with a further excitation, that is possible over three resonant energy potential curves into the ionic ground-state. In the second part of my thesis I realized pump-probe spectroscopy of Rb{sub 2} dimers in a dark SPOT. (orig.)

Pulse shape and spectrum of coherent diffraction-limited transition radiation from electron beams

Energy Technology Data Exchange (ETDEWEB)

van Tilborg, J.; Schroeder, C.B.; Esarey, E.; Leemans, W.P.

2003-12-20

The electric field in the temporal and spectral domain of coherent diffraction-limited transition radiation is studied. An electron bunch, with arbitrary longitudinal momentum distribution, propagating at normal incidence to a sharp metal-vacuum boundary with finite transverse dimension is considered. A general expression for the spatiotemporal electric field of the transition radiation is derived, and closed-form solutions for several special cases are given. The influence of parameters such as radial boundary size, electron momentum distribution, and angle of observation on the waveform (e.g., radiation pulse length and amplitude) are discussed. For a Gaussian electron bunch, the coherent radiation waveform is shown to have a single-cycle profile. Application to a novel THz source based on a laser-driven accelerator is discussed.

Diode-pumped solid state laser. (Part V). ; Short pulse laser oscillation. Handotai laser reiki kotai laser. 5. ; Tan pulse hasshin

Energy Technology Data Exchange (ETDEWEB)

Kuwabara, M.; Bando, N. (Asahi Glass Co. Ltd., Tokyo (Japan))

1991-12-25

A semiconductor laser (LD) excited solid state laser using an LD as an excited light source is under discussion for its practical applications to measurements, processing, communications, office automation, and medical areas. This paper describes the discussions given on the short pulse transmission using AOQ switching elements in the LD excited solid state laser with a long wave length band (1.3{mu}m), which is expected of its application in the communications and measurements area. Based on a possibility of raising a measurements resolution by making the pluses in the LD excited solid state laser, and experiments were performed using Nd:YLF as a laser host. as a results, it was found that the smaller the effective mode volume V {sub eff},the smaller the pulse width, and that the ratio of number of initial inversion distribution (N{sub i}/N{sub t}), an important parameter to determine pulse widths, can be obtained from the ratio of the LD exciting light to the input power (P{sub in}/P{sub t}). 7 refs., 14 figs., 2 tabs.

Coherent control of atoms and diatomic molecules with shaped ultrashort pulses

International Nuclear Information System (INIS)

Degert, J.

2002-12-01

This thesis deals with the theoretical and experimental study of coherent control of atomic and molecular systems with shaped pulses. At first, we present several experiments of control of coherent transients in rubidium. These transients appear when a two-level system is excited by a perturbative chirped pulse, and are characterized by oscillations in the excited state population. For a strong chirp, we show that a phase step in the spectrum modifies the phase of the oscillations. Then, by direct analogy with Fresnel zone lens, we conceive a chirped pulse with a highly modulated amplitude, allowing to suppress destructive contributions to the population transfer. In a second set of experiments, we focus on quantum path interferences in two-photon transitions excited by linearly chirped pulses. Owing to the broad bandwidth of ultrashort pulses, sequential and direct excitation paths contribute to the excited state population. Oscillations resulting from interferences between these two paths are observed in atomic sodium. Moreover, we show that they are observable whatever the sign of chirp. Theoretically, we study the control of the predissociation of a benchmark diatomic molecule: NaI. Predissociation leads to matter wave interferences in the fragments distribution. First, we show that a suitably chosen probe pulse allows the observation of theses interferences. Next, using a sequence of control pulse inducing electronic transition, we demonstrate the possibility to manipulate fragment energy distribution. (author)

Laser ablation comparison by picosecond pulses train and nanosecond pulse

Science.gov (United States)

Lednev, V. N.; Filippov, M. N.; Bunkin, A. F.; Pershin, S. M.

2015-12-01

A comparison of laser ablation by a train of picosecond pulses and nanosecond pulses revealed a difference in laser craters, ablation thresholds, plasma sizes and spectral line intensities. Laser ablation with a train of picosecond pulses resulted in improved crater quality while ablated mass decreased up to 30%. A reduction in laser plasma dimensions for picosecond train ablation was observed while the intensity of atomic/ionic lines in the plasma spectra was greater by a factor of 2-4 indicating an improved excitation and atomization in the plasma.

Temporal evolution of atmosphere pressure plasma jets driven by microsecond pulses with positive and negative polarities

Science.gov (United States)

Shao, Tao; Yang, Wenjin; Zhang, Cheng; Fang, Zhi; Zhou, Yixiao; Schamiloglu, Edl

2014-09-01

Current-voltage characteristics, discharge images, and optical spectra of atmospheric pressure plasma jets (APPJs) are studied using a microsecond pulse length generator producing repetitive output pulses with different polarities. The experimental results show that the APPJs excited by the pulses with positive polarity have longer plume, faster propagation speed, higher power, and more excited species, such as \\text{N}2 , O, He, \\text{N}2+ , than that with the negatively excited APPJs. The images taken using an intensified charge-coupled device show that the APPJs excited by pulses with positive polarity are characterized by a bullet-like structure, while the APPJs excited by pulses with negative polarity are continuous. The propagation speed of the APPJs driven by a microsecond pulse length generator is about tens of km/s, which is similar to the APPJs driven by a kHz frequency sinusoidal voltage source. The analysis shows that the space charge accumulation effect plays an important role during the discharge. The transient enhanced electric field induced by the accumulated ions between the needle-like electrode and the nozzle in the APPJs excited by pulses with negative polarity enhances electron field emission from the cathode, which is illustrated by the bright line on the time-integrated images. This makes the shape of the APPJ excited using pulses with negative polarity different from the bullet-like shape of the APPJs excited by pulses with positive polarity.

Comparison of high-voltage ac and pulsed operation of a surface dielectric barrier discharge

Energy Technology Data Exchange (ETDEWEB)

Williamson, James M [Innovative Scientific Solutions, Inc., 2766 Indian Ripple Road, Dayton, Ohio 45440-3638 (United States); Trump, Darryl D [Innovative Scientific Solutions, Inc., 2766 Indian Ripple Road, Dayton, Ohio 45440-3638 (United States); Bletzinger, Peter [Innovative Scientific Solutions, Inc., 2766 Indian Ripple Road, Dayton, Ohio 45440-3638 (United States); Ganguly, Biswa N [Air Force Research Laboratory, Wright-Patterson Air Force Base, Ohio 45433-7919 (United States)

2006-10-21

A surface dielectric barrier discharge (DBD) in atmospheric pressure air was excited either by low frequency (0.3-2 kHz) high-voltage ac or by short, high-voltage pulses at repetition rates from 50 to 600 pulses s{sup -1}. The short-pulse excited discharge was more diffuse and did not have the pronounced bright multiple cathode spots observed in the ac excited discharge. The discharge voltage, current and average power deposited into the discharge were calculated for both types of excitation. As a measure of plasma-chemical efficiency, the ozone number density was measured by UV absorption as a function of average deposited power. The density of ozone produced by ac excitation did not increase so rapidly as that produced by short-pulse excitation as a function of average power, with a maximum measured density of {approx}3 x 10{sup 15} cm{sup -3} at 25 W. The maximum ozone production achieved by short-pulse excitation was {approx}8.5 x 10{sup 15} cm{sup -3} at 20 W, which was four times greater than that achieved by ac excitation at the same power level.

Comparison of high-voltage ac and pulsed operation of a surface dielectric barrier discharge

International Nuclear Information System (INIS)

Williamson, James M; Trump, Darryl D; Bletzinger, Peter; Ganguly, Biswa N

2006-01-01

A surface dielectric barrier discharge (DBD) in atmospheric pressure air was excited either by low frequency (0.3-2 kHz) high-voltage ac or by short, high-voltage pulses at repetition rates from 50 to 600 pulses s -1 . The short-pulse excited discharge was more diffuse and did not have the pronounced bright multiple cathode spots observed in the ac excited discharge. The discharge voltage, current and average power deposited into the discharge were calculated for both types of excitation. As a measure of plasma-chemical efficiency, the ozone number density was measured by UV absorption as a function of average deposited power. The density of ozone produced by ac excitation did not increase so rapidly as that produced by short-pulse excitation as a function of average power, with a maximum measured density of ∼3 x 10 15 cm -3 at 25 W. The maximum ozone production achieved by short-pulse excitation was ∼8.5 x 10 15 cm -3 at 20 W, which was four times greater than that achieved by ac excitation at the same power level

Dynamics of electron solvation in methanol: Excited state relaxation and generation by charge-transfer-to-solvent

International Nuclear Information System (INIS)

Elkins, Madeline H.; Williams, Holly L.; Neumark, Daniel M.

2015-01-01

The charge-transfer-to-solvent dynamics (CTTS) and excited state relaxation mechanism of the solvated electron in methanol are studied by time-resolved photoelectron spectroscopy on a liquid methanol microjet by means of two-pulse and three-pulse experiments. In the two-pulse experiment, CTTS excitation is followed by a probe photoejection pulse. The resulting time-evolving photoelectron spectrum reveals multiple time scales characteristic of relaxation and geminate recombination of the initially generated electron which are consistent with prior results from transient absorption. In the three-pulse experiment, the relaxation dynamics of the solvated electron following electronic excitation are measured. The internal conversion lifetime of the excited electron is found to be 130 ± 40 fs, in agreement with extrapolated results from clusters and the non-adiabatic relaxation mechanism

Dynamics of electron solvation in methanol: Excited state relaxation and generation by charge-transfer-to-solvent

Science.gov (United States)

Elkins, Madeline H.; Williams, Holly L.; Neumark, Daniel M.

2015-06-01

The charge-transfer-to-solvent dynamics (CTTS) and excited state relaxation mechanism of the solvated electron in methanol are studied by time-resolved photoelectron spectroscopy on a liquid methanol microjet by means of two-pulse and three-pulse experiments. In the two-pulse experiment, CTTS excitation is followed by a probe photoejection pulse. The resulting time-evolving photoelectron spectrum reveals multiple time scales characteristic of relaxation and geminate recombination of the initially generated electron which are consistent with prior results from transient absorption. In the three-pulse experiment, the relaxation dynamics of the solvated electron following electronic excitation are measured. The internal conversion lifetime of the excited electron is found to be 130 ± 40 fs, in agreement with extrapolated results from clusters and the non-adiabatic relaxation mechanism.

Dynamics of electron solvation in methanol: Excited state relaxation and generation by charge-transfer-to-solvent

Energy Technology Data Exchange (ETDEWEB)

Elkins, Madeline H.; Williams, Holly L. [Department of Chemistry, University of California, Berkeley, California 94720 (United States); Neumark, Daniel M. [Department of Chemistry, University of California, Berkeley, California 94720 (United States); Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States)

2015-06-21

The charge-transfer-to-solvent dynamics (CTTS) and excited state relaxation mechanism of the solvated electron in methanol are studied by time-resolved photoelectron spectroscopy on a liquid methanol microjet by means of two-pulse and three-pulse experiments. In the two-pulse experiment, CTTS excitation is followed by a probe photoejection pulse. The resulting time-evolving photoelectron spectrum reveals multiple time scales characteristic of relaxation and geminate recombination of the initially generated electron which are consistent with prior results from transient absorption. In the three-pulse experiment, the relaxation dynamics of the solvated electron following electronic excitation are measured. The internal conversion lifetime of the excited electron is found to be 130 ± 40 fs, in agreement with extrapolated results from clusters and the non-adiabatic relaxation mechanism.

Native protein excited by low doses of γ-radiation serves as a source of secondary biogenic radiation

International Nuclear Information System (INIS)

Kuzin, A.M.; Surkenova, G.N.; Revin, A.F.

1996-01-01

In is demonstrated that native protein of egg-white after being γ-irradiated with law doses is able to stimulate transition of cells of remote biological detector from non-cycling state to proliferation even if irradiated protein is separated from detector by quartz-glass. Animal tissues which have a high protein content (freshly cut hair, insect bodies) reveal the same ability. The role of natural background radiation in the maintenance excitation, state of living tissue proteins is discussed. 13 refs.; 1 figs.; 4 tabs

Reduction of CSF flow artifact in fast fluid attenuated inversion recovery MR imaging. Study of excitation width in 180deg inversion pulse

International Nuclear Information System (INIS)

Tsuchihashi, Toshio; Yoshizawa, Satoshi; Maki, Toshio; Kitagawa, Matsuo; Suzuki, Ken; Fujita, Isao

1998-01-01

A technique that increases slice thickness so that it becomes wider than the excitation width of the 180deg inversion pulse and in which TR is partitioned twice has been investigated with regard to fast FLAIR. This is a technique that reduces the flow artifact of CSF. It is thought that, with this technique, the flow artifact is reduced because the CSF that flows onto the slice reaches the null point. The cross talk effect of the 180deg inversion pulse appears as a high CSF signal. As a result, the number of slices needs to be partitioned two or three times before imaging. Thus the imaging time is doubled or tripled. Considering the cross talk effect of the 180deg inversion pulse and the imaging time needed for this technique, the optimal imaging technique would be one that uses an inversion pulse that is four times slice thickness plus slice space and for which the number of slices is partitioned twice. Furthermore, the null point of CSF was dependent on dividing TR in half. (author)

Synchrotron radiation excited silicon epitaxy using disilane

International Nuclear Information System (INIS)

Akazawa, Housei; Utsumi, Yuichi

1995-01-01

Synchrotron radiation (SR) excited chemical reactions provide new crystal growth methods suitable for low-temperature Si epitaxy. The growth kinetics and film properties were investigated by atomic layer epitaxy (ALE) and photochemical vapor deposition (CVD) modes using Si 2 H 6 . SR-ALE, isolating the surface growth channel mediated by photon stimulated hydrogen desorption, achieves digital growth independent of gas exposure time, SR irradiation time, and substrate temperature. On the other hand in SR-CVD, photolysis of Si 2 H 6 is predominant. In the nonirradiated region, Eley-Rideal type reaction between the photofragments and the surface deposit Si adatoms in a layer-by-layer fashion. In the irradiated region, however, multi-layer photolysis and rebounding occurs within the condensed Si 2 H 6 layer. The pertinent elementary processes were identified by using the high-resolution time-of-flight mass spectroscopy. The SR-CVD can grow a uniform and epitaxial Si film down to 200degC. The surface morphology is controlled by the surfactant effect of hydrogen atoms. (author)

Dose measurements in pulsed radiation fields with commercially available measuring components

International Nuclear Information System (INIS)

Friedrich, Sabrina; Hupe, Oliver

2016-01-01

Dose measurements in pulsed radiation fields with dosemeters using the counting technique are known to be inappropriate. Therefore, there is a demand for a portable device able to measure the dose in pulsed radiation fields. As a detector, ionisation chambers seem to be a good alternative. In particular, using a secondary standard ionisation chamber in combination with a reliable charge-measuring system would be a good solution. The Physikalisch-Technische Bundesanstalt (PTB) uses secondary standard ionisation chambers in combination with PTB-made measuring electronics for dose measurements at its reference fields. However, for general use, this equipment is too complex. For measurements on-site, a mobile special electronic system [Hupe, O. and Ankerhold, U. Determination of ambient and personal dose equivalent for personnel and cargo security screening. Radiat. Prot. Dosim. 121(4), 429-437 (2006)] has been used successfully. Still, for general use, there is a need for a much simpler but a just as good solution. A measuring instrument with very good energy dependence for H*(10) is the secondary standard ionisation chamber HS01. An easy-to-use and commercially available electrometer for measuring the generated charges is the UNIDOS by PTW Freiburg. Depending on the expected dose values, the ionisation chamber used can be selected. In addition, measurements have been performed by using commercially available area dosemeters, e.g. the Mini SmartION 2120S by Thermo Scientific, using an ionisation chamber and the Szintomat 6134 A/H by Automess, using a scintillation detector. (authors)

Foot-pulse radiation drive necessary for ICF ignition capsule demonstrated on Z generator

International Nuclear Information System (INIS)

Sanford, T.W.L.; Olson, R.E.; Chandler, G.A.

1999-01-01

Implosion and ignition of an indirectly-driven ICF capsule operating near a Fermi-degenerate isentrope requires initial Planckian-radiation-drive temperatures of 70-to-90 eV to be present for a duration of 10-to-15 ns prior to the main drive pulse. Such capsules are being designed for high pulsed-power generators. This foot-pulse drive capability has been recently demonstrated in a NIF-sized (φ = 6-mm 1 = 7-mm), gold hohlraum, using a one-sided static-wall hohlraum geometry on the Z generator. The general arrangement utilized nested tungsten-wire arrays of radii (mass) 20 mm (2 mg) and 10 mm (1 mg) that had an axial length of approximately 10 mm. The arrays were driven by a peak current of approximately 21 MA and were made to implode on a 2-microm-thick Cu annulus (mass = 4.5 mg), which had a radius of 4 mm and was filled with a low-density CH foam, all centered about the z-axis. The gold hohlraum was mounted on axis and above the Cu/foam target. A 2.9-mm-radius axial hole between the top of the target and hohlraum permitted the x-rays generated from the implosion to enter the hohlraum. The radiation within the hohlraum was monitored by viewing the hohlraum through a 3-mm diameter hole on the lateral side of the hohlraum with a suite of diagnostics.The radiation entering the hohlraum was estimated by an additional suite of on-axis diagnostics, in a limited number of separate shots, when the hohlraum was not present. Additionally, the radiation generated outside the Cu annulus was monitored, for all shots, through a 3-mm diameter aperture located on the outside of the current return can. In the full paper, the characteristics of the radiation measured from these diagnostic sets, including the Planckian temperature of the hohlraum and radiation images, will be discussed as a function of the incident wire-array geometry (single vs nested array and array mass), target length (10, or 20 mm), annulus material (Cu, Au, or nothing), and CH-foam-fill density (10, 6, 2

Study of phonon-induced energy transfer processes in crystals using heat pulses

International Nuclear Information System (INIS)

Burns, A.R.

1978-03-01

The artificial generation of acoustic lattice vibrations by a heat pulse technique is developed in order to probe phonon interactions in molecular crystals. Specifically, the phonon-assisted delocalization of ''trapped'' excited triplet state energy in the aromatic crystal 1,2,4,5-tetrachlorobenzene (TCB) is studied in a quantitative manner by monitoring the time-resolved decrease in trap phosphorescence intensity due to the propagation of a well-defined heat pulse. The excitation distribution in a single trap system, such as the X-trap in neat h 2 -TCB, is discussed in terms of the energy partition function relating the temperature dependence of the trap phosphorescence intensity to the trap depth, exciton bandwidth, and the number of exciton band states. In a multiple trap system, such as the hd and h 2 isotopic traps in d 2 -TCB, the excitation distribution is distinctly non-Boltzmann; yet it may be discussed in terms of a preferential energy transfer between the two trap states via the exciton band. For both trap systems, a previously developed kinetic model is presented which relates the efficiency of trap-band energy exchange to the density of band states and the trap-phonon coupling matrix elements. A bolometric technique for determining the thermal response time of the heater/crystal system is presented. The phonon mean free path in the crystal is size-limited, and the heater/crystal boundary conductance is reasonably close to previously reported values. The theory of heat pulse phonon spectroscopy is presented and discussed in terms of black-body phonon radiation

The accumulation of femtosecond laser radiation energy in crystals of lithium fluoride

Science.gov (United States)

Dresvyanskiy, V. P.; Glazunov, D. S.; Alekseev, S. V.; Losev, V. F.; Chadraa, B.; Bukhtsooj, O.; Baasankhuu, N.; Zandan, B.; Martynovich, E. F.

2015-12-01

We present the results of studies of energy accumulation during the non-destructive interaction of extremely intense near infrared laser radiation with model wide band gap dielectric crystals of lithium fluoride, when the intensity of pulses is sufficient for effective highly nonlinear absorption of light and for the excitation of the electron subsystem of matter and the energy of pulses is still not sufficient for significant heating, evaporation, laser breakdown or other destruction to occur. We studied the emission of energy in the form of light sum of thermally stimulated luminescence accumulated under conditions of self-focusing and multiple filamentation of femtosecond laser radiation. It was established that it's the F2 and F3+ color centers and supplementary to them centers of interstitial type which accumulate energy under the action of a single femtosecond laser pulses. When irradiated by series of pulses the F3, F3- and F4 centers additionally appear. F2 centers are the main centers of emission in the process of thermally stimulated luminescence of accumulated energy. The interstitial fluoride ions (I-centers) are the kinetic particles. They split off from the X3- centers in the result of thermal decomposition of latter on the I-centers and molecules X20. I-centers recombine with F3+ centers and form F2 centers in excited state. The latter produce the characteristic emission spectrum emitted in the form of thermally stimulated luminescence.

Effect resonance radiation transfer of excitation porous silicon to I sub 2 molecules sorbed in pores

CERN Document Server

Zakharchenko, K V; Kuznetsov, M B; Chistyakov, A A; Karavanskij, V A

2001-01-01

One studies the effect of resonance radiation-free transfer of electronic excitation between silicon nanocrystals and iodine molecules sorbed in pores. The experiment procedure includes laser-induced luminescence and laser desorption mass spectrometry. One analyzes photoluminescence spectra prior to and upon iodine sorption. Excitation of iodine through the mechanism of resonance transfer is determined to result in desorption of the iodine sorbed molecules with relatively high kinetic energies (3-1 eV). One evaluated the peculiar distance of resonance transfer the approximate value of which was equal to 2 nm

Simulation of pulsed-ionizing-radiation-induced errors in CMOS memory circuits

International Nuclear Information System (INIS)

Massengill, L.W.

1987-01-01

Effects of transient ionizing radiation on complementary metal-oxide-semiconductor (CMOS) memory circuits was studied by computer simulation. Simulation results have uncovered the dominant mechanism leading to information loss (upset) in dense (CMOS) circuits: rail span collapse. This effect is the catastrophic reduction in the local power supply at a RAM cell location due to the conglomerate radiation-induced photocurrents from all other RAM cells flowing through the power-supply-interconnect distribution. Rail-span collapse leads to reduced RAM cell-noise margins and can predicate upset. Results show that rail-span collapse in the dominant pulsed radiation effect in many memory circuits, preempting local circuit responses to the radiation. Several techniques to model power-supply noise, such as that arising from rail span collapse, are presented in this work. These include an analytical model for design optimization against these effects, a hierarchical computer-analysis technique for efficient power bus noise simulation in arrayed circuits, such as memories, and a complete circuit-simulation tool for noise margin analysis of circuits with arbitrary topologies

Dependence of the absorption of pulsed CO2-laser radiation by silane on wavenumber, fluence, pulse duration, temperature, optical path length, and pressure of absorbing and nonabsorbing gases

International Nuclear Information System (INIS)

Blazejowski, J.; Gruzdiewa, L.; Rulewski, J.; Lampe, F.W.

1995-01-01

The absorption of three lines [P(20), 944.2 cm -1 ; P(14), 949.2 cm -1 ; and R(24), 978.5 cm -1 ] of the pulsed CO 2 laser (00 0 1--10 0 0 transition) by SiH 4 was measured at various pulse energy, pulse duration, temperature, optical path length, and pressure of the compound and nonabsorbing foreign gases. In addition, low intensity infrared absorption spectrum of silane was compared with high intensity absorption characteristics for all lines of the pulsed CO 2 laser. The experimental dependencies show deviations from the phenomenological Beer--Lambert law which can be considered as arising from the high intensity of an incident radiation and collisions of absorbing molecules with surroundings. These effects were included into the expression, being an extended form of the Beer--Lambert law, which reasonably approximates all experimental data. The results, except for extending knowledge on the interaction of a high power laser radiation with matter, can help understanding and planning processes leading to preparation of silicon-containing technologically important materials

New method to measure the angular antispring effect in a Fabry–Perot cavity with remote excitation using radiation pressure

Energy Technology Data Exchange (ETDEWEB)

Nagano, Koji, E-mail: knagano@icrr.u-tokyo.ac.jp [Institute for Cosmic Ray Research, The University of Tokyo, 5-1-5 Kashiwa-no-Ha, Kashiwa, Chiba 277-8582 (Japan); Enomoto, Yutaro; Nakano, Masayuki [Institute for Cosmic Ray Research, The University of Tokyo, 5-1-5 Kashiwa-no-Ha, Kashiwa, Chiba 277-8582 (Japan); Furusawa, Akira [Department of Applied Physics, School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656 (Japan); Kawamura, Seiji [Institute for Cosmic Ray Research, The University of Tokyo, 5-1-5 Kashiwa-no-Ha, Kashiwa, Chiba 277-8582 (Japan)

2016-03-06

In experiments with Fabry–Perot cavities consisting of suspended mirrors, an angular antispring effect on the mirror of the cavity is caused by radiation pressure from resonant light in the cavity. A new method was invented to measure the effect precisely with remote excitation on the mirror using the radiation pressure. This method was found to be available for the suspended 23 mg mirror and improved the measurement accuracy by a factor of two, compared with the previous method. This result leads to stable control systems to eliminate the angular instability of the mirror caused by the effect. - Highlights: • A method to measure an angular antispring effect on a suspended mirror was proposed. • Remote excitation on the mirror with radiation pressure of resonant light is used. • This method provides better measurement accuracy compared with the previous method.

Using a heterodyne vibrometer in combination with pulse excitation for primary calibration of ultrasonic hydrophones in amplitude and phase

Science.gov (United States)

Weber, Martin; Wilkens, Volker

2017-08-01

A high-frequency vibrometer was used with ultrasonic pulse excitation in order to perform a primary hydrophone calibration. This approach enables the simultaneous characterization of the amplitude and phase transfer characteristic of ultrasonic hydrophones. The method allows a high frequency resolution in a considerably short time for the measurement. Furthermore, the uncertainty contributions of this approach were investigated and quantified. A membrane hydrophone was calibrated and the uncertainty budget for this measurement was determined. The calibration results are presented up to 70~\\text{MHz} . The measurement results show good agreement with the results obtained by sinusoidal burst excitation through the use of the vibrometer and by a homodyne laser interferometer, with RMS deviation of approximately 3% -4% in the frequency range from 1 to 60~\\text{MHz} . Further hydrophones were characterized up to 100~\\text{MHz} with this procedure to demonstrate the suitability for very high frequency calibration.

Stimulated emission depletion following two photon excitation

OpenAIRE

Marsh, R. J.; Armoogum, D. A.; Bain, A. J.

2002-01-01

The technique of stimulated emission depletion of fluorescence (STED) from a two photon excited molecular population is demonstrated in the S, excited state of fluorescein in ethylene glycol and methanol. Two photon excitation (pump) is achieved using the partial output of a regeneratively amplified Ti:Sapphire laser in conjunction with an optical parametric amplifier whose tuneable output provides a synchronous depletion (dump) pulse. Time resolved fluorescence intensity and anisotropy measu...

Pulse power technology application to lasers

International Nuclear Information System (INIS)

Prestwich, K.R.

1975-01-01

Recent developments of intense relativistic electron beam accelerators and the associated pulse power technology are reviewed. The design of specific accelerators for gas laser excitation sources is discussed. A 3 MV, 800 kA, 24 ns electron beam accelerator under development for the electron beam fusion program is described along with the low jitter multichannel oil-dielectric rail switches developed for this application. This technology leads to the design of a 20 kJ, short pulse accelerator optimized gas laser excitation with radially converging electron beams. Other gas laser research requirements have led to the development of an accelerator that will produce a 0.5 MV, 20 kJ, 1 μs electron beam pulse. (auth)

A conceptual design of the set-up for solid state spectroscopy with free electron laser and insertion device radiation

CERN Document Server

Makhov, V N

2001-01-01

The set-up for complex solid state spectroscopy with the use of enhanced properties of radiation from insertion devices and free electron lasers is proposed. Very high flux and pulsed properties of radiation from insertion devices and free electron lasers offer the possibility for the use of such powerful techniques as electron paramagnetic resonance (EPR) and optically detected magnetic resonance (ODMR) for the studies of excited states of electronic excitations or defects in solids. The power density of radiation can become high enough for one more method of exited-state spectroscopy: transient optical absorption spectroscopy. The set-up is supposed to combine the EPR/ODMR spectrometer, i.e. cryostat supplied with superconducting magnet and microwave system, and the optical channels for excitation (by radiation from insertion devices or free electron laser) and detection of luminescence (i.e. primary and secondary monochromators). The set-up can be used both for 'conventional' spectroscopy of solids (reflec...

Quantum deformation of the angular distributions of synchrotron radiation. Emission from particles in the first excited state

Energy Technology Data Exchange (ETDEWEB)

Bagrov, V.G. [Tomsk State University, Department of Physics, Tomsk (Russian Federation); SB RAS, Tomsk Institute of High Current Electronics, Tomsk (Russian Federation); University of Sao Paulo, Institute of Physics, Sao Paulo (Brazil); Burimova, A.N. [Tomsk State University, Department of Physics, Tomsk (Russian Federation); University of Sao Paulo, Institute of Physics, Sao Paulo (Brazil); Gitman, D.M.; Levin, A.D. [University of Sao Paulo, Institute of Physics, Sao Paulo (Brazil)

2012-02-15

The exact expressions for the characteristics of synchrotron radiation of charged particles in the first excited state are obtained in analytical form using quantum theory methods. We performed a detailed analysis of the angular distribution structure of radiation power and its polarization for particles with spin 0 and 1/2. It is shown that the exact quantum calculations lead to results that differ substantially from the predictions of classical theory. (orig.)

Integrated light in direct excitation and energy transfer luminescence

OpenAIRE

Chimczak, Eugeniusz

2007-01-01

Integrated light in direct excitation and energy transfer luminescence has been investigated. In the investigations reported here, monomolecular centers were taken into account. It was found that the integrated light is equal to the product of generation rate and time of duration of excitation pulse for both direct excitation and energy transfer luminescence.

Even-parity resonances with synchrotron radiation from Laser Excited Lithium at 1s^22p State

Science.gov (United States)

Huang, Ming-Tie; Wehlitz, Ralf

2010-03-01

Correlated many-body dynamics is still one of the unsolved fundamental problems in physics. Such correlation effects can be most clearly studied in processes involving single atoms for their simplicity.Lithium, being the simplest open shell atom, has been under a lot of study. Most of the studies focused on ground state lithium. However, only odd parity resonances can be populated through single photon (synchrotron radiation) absorption from ground state lithium (1s^22s). Lithium atoms, after being laser excited to the 1s^22p state, allow the study of even parity resonances. We have measured some of the even parity resonances of lithium for resonant energies below 64 eV. A single-mode diode laser is used to excite lithium from 1s^22s ground state to 1s^22p (^2P3/2) state. Photoions resulting from the interaction between the excited lithium and synchrotron radiation were analyzed and collected by an ion time-of-flight (TOF) spectrometer with a Z- stack channel plate detector. The Li^+ ion yield was recorded while scanning the undulator along with the monochromator. The energy scans have been analyzed regarding resonance energies and parameters of the Fano profiles. Our results for the observed resonances will be presented.

Photoionization pathways and thresholds in generation of Lyman-α radiation by resonant four-wave mixing in Kr-Ar mixture

Directory of Open Access Journals (Sweden)

Oleg A. Louchev

2016-09-01

Full Text Available We develop a set of analytical approximations for the estimation of the combined effect of various photoionization processes involved in the resonant four-wave mixing generation of ns pulsed Lyman-α (L-α radiation by using 212.556 nm and 820-845 nm laser radiation pulses in Kr-Ar mixture: (i multi-photon ionization, (ii step-wise (2+1-photon ionization via the resonant 2-photon excitation of Kr followed by 1-photon ionization and (iii laser-induced avalanche ionization produced by generated free electrons. Developed expressions validated by order of magnitude estimations and available experimental data allow us to identify the area for the operation under high input laser intensities avoiding the onset of full-scale discharge, loss of efficiency and inhibition of generated L-α radiation. Calculations made reveal an opportunity for scaling up the output energy of the experimentally generated pulsed L-α radiation without significant enhancement of photoionization.

Photoionization pathways and thresholds in generation of Lyman-α radiation by resonant four-wave mixing in Kr-Ar mixture

Science.gov (United States)

Louchev, Oleg A.; Saito, Norihito; Oishi, Yu; Miyazaki, Koji; Okamura, Kotaro; Nakamura, Jumpei; Iwasaki, Masahiko; Wada, Satoshi

2016-09-01

We develop a set of analytical approximations for the estimation of the combined effect of various photoionization processes involved in the resonant four-wave mixing generation of ns pulsed Lyman-α (L-α ) radiation by using 212.556 nm and 820-845 nm laser radiation pulses in Kr-Ar mixture: (i) multi-photon ionization, (ii) step-wise (2+1)-photon ionization via the resonant 2-photon excitation of Kr followed by 1-photon ionization and (iii) laser-induced avalanche ionization produced by generated free electrons. Developed expressions validated by order of magnitude estimations and available experimental data allow us to identify the area for the operation under high input laser intensities avoiding the onset of full-scale discharge, loss of efficiency and inhibition of generated L-α radiation. Calculations made reveal an opportunity for scaling up the output energy of the experimentally generated pulsed L-α radiation without significant enhancement of photoionization.

Comparison of pulsed fluoroscopy by direct control using a grid-controlled x-ray tube with pulsed fluoroscopy by primary control

International Nuclear Information System (INIS)

Chida, Koichi; Zuguchi, Masayuki; Ito, Daisuke; Sato, Kunihiko; Shimura, Hirotaka; Sasaki, Masatoshi

2001-01-01

Interventional radiology (IVR) procedures may involve high radiation doses that are potentially harmful to the patient. In IVR procedures, pulsed fluoroscopy can greatly decrease the radiation that the physician and patient receive. There are two types of pulsed fluoroscopy: direct control and primary (indirect) control. The purpose of this study was to compare pulsed fluoroscopy by direct control, using a grid-controlled x-ray tube, with pulsed fluoroscopy using primary control. For both types of pulsed fluoroscopy, we measured the waveforms (x-ray tube voltage, x-ray tube current, and x-ray output) and the relative radiation dose. In addition, we compared the decrease in radiation during pulsed fluoroscopy using a care filter. The studies were performed using a Siemens Bicor Plus x-ray System (direct control) and a Siemens Multistar Plus x-ray System (primary control). Using primary pulse control, a 50% decrease in the x-ray output waveform took approximately 0.5-1.0 msec, or longer with a lower x-ray tube current. Using direct pulse control, a 50% decrease in the x-ray output waveform took approximately 0.1 msec, and was independent of x-ray tube current. The rate of radiation reduction with primary pulse control using the care filter with a lower x-ray tube current had a slope exceeding 10%. Pulsed fluoroscopy by direct control using a grid-controlled x-ray tube permits an optimal radiation dose. To decrease the radiation in primary pulse control, a care filter must be used, particularly with a lower x-ray tube current. (author)

Detection of leak-defective fuel rods using the circumferential Lamb waves excited by the resonance backscattering of ultrasonic pulses

International Nuclear Information System (INIS)

Choi, M.S.; Yang, M.S.; Kim, H.C.

1992-01-01

A new ultrasonic technique for detecting the infiltrated water in leaked fuel rods is developed. Propagation characteristics of the circumferential Lamb waves in the cladding tubes are estimated by the resonance scattering theory. The Lamb waves are excited by the resonance backscattering of ultrasonic pulses. In sound fuel rods, the existence of the Lamb waves is revealed by a series of periodic echoes. In leaked fuel rods, however, the Lamb waves are perturbed strongly by the scattered waves from the surface of fuel pellets, thus the periodic echoes are not observed. (author)

INTERACTION OF LASER RADIATION WITH MATTER: Influence of a target on operation of a pulsed CO2 laser emitting microsecond pulses

Science.gov (United States)

Baranov, V. Yu; Dolgov, V. A.; Malyuta, D. D.; Mezhevov, V. S.; Semak, V. V.

1987-12-01

The profile of pulses emitted by a TEA CO2 laser with an unstable resonator changed as a result of interaction of laser radiation with the surface of a metal in the presence of a breakdown plasma. This influence of a target on laser operation and its possible applications in laser processing of materials are analyzed.

Photofragmentation of colloidal solutions of gold nanoparticles under femtosecond laser pulses in IR and visible ranges

International Nuclear Information System (INIS)

Danilov, P A; Zayarnyi, D A; Ionin, A A; Kudryashov, S I; Makarov, S V; Rudenko, A A; Saraeva, I N; Yurovskikh, V I; Lednev, V N; Pershin, S M

2015-01-01

The specific features of photofragmentation of sols of gold nanoparticles under focused femtosecond laser pulses in IR (1030 nm) and visible (515 nm) ranges is experimentally investigated. A high photofragmentation efficiency of nanoparticles in the waist of a pulsed laser beam in the visible range (at moderate radiation scattering) is demonstrated; this efficiency is related to the excitation of plasmon resonance in nanoparticles on the blue shoulder of its spectrum, in contrast to the regime of very weak photofragmentation in an IR-laser field of comparable intensity. Possible mechanisms of femtosecond laser photofragmentation of gold nanoparticles are discussed. (extreme light fields and their applications)

Standard Test Method for Measuring Dose for Use in Linear Accelerator Pulsed Radiation Effects Tests

CERN Document Server

American Society for Testing and Materials. Philadelphia

2011-01-01

1.1 This test method covers a calorimetric measurement of the total dose delivered in a single pulse of electrons from an electron linear accelerator or a flash X-ray machine (FXR, e-beam mode) used as an ionizing source in radiation-effects testing. The test method is designed for use with pulses of electrons in the energy range from 10 to 50 MeV and is only valid for cases in which both the calorimeter and the test specimen to be irradiated are“thin” compared to the range of these electrons in the materials of which they are constructed. 1.2 The procedure described can be used in those cases in which (1) the dose delivered in a single pulse is 5 Gy (matl) (500 rd (matl)) or greater, or (2) multiple pulses of a lower dose can be delivered in a short time compared to the thermal time constant of the calorimeter. Matl refers to the material of the calorimeter. The minimum dose per pulse that can be acceptably monitored depends on the variables of the particular test, including pulse rate, pulse uniformity...

Measuring radiation damage dynamics by pulsed ion beam irradiation: 2016 project annual report

Energy Technology Data Exchange (ETDEWEB)

Kucheyev, Sergei O. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

2017-01-04

The major goal of this project is to develop and demonstrate a novel experimental approach to access the dynamic regime of radiation damage formation in nuclear materials. In particular, the project exploits a pulsed-ion-beam method in order to gain insight into defect interaction dynamics by measuring effective defect interaction time constants and defect diffusion lengths. For Year 3, this project had the following two major milestones: (i) the demonstration of the measurement of thermally activated defect-interaction processes by pulsed ion beam techniques and (ii) the demonstration of alternative characterization techniques to study defect dynamics. As we describe below, both of these milestones have been met.

Laser amplification in excited dielectrics

Science.gov (United States)

Winkler, Thomas; Haahr-Lillevang, Lasse; Sarpe, Cristian; Zielinski, Bastian; Götte, Nadine; Senftleben, Arne; Balling, Peter; Baumert, Thomas

2018-01-01

Wide-bandgap dielectrics such as glasses or water are transparent at visible and infrared wavelengths. This changes when they are exposed to ultrashort and highly intense laser pulses. Different interaction mechanisms lead to the appearance of various transient nonlinear optical phenomena. Using these, the optical properties of dielectrics can be controlled from the transparent to the metal-like state. Here we expand this range by a yet unexplored mechanism in excited dielectrics: amplification. In a two-colour pump-probe experiment, we show that a 400 nm femtosecond laser pulse is coherently amplified inside an excited sapphire sample on a scale of a few micrometres. Simulations strongly support the proposed two-photon stimulated emission process, which is temporally and spatially controllable. Consequently, we expect applications in all fields that demand strongly localized amplification.

Pulsed neutron well logging apparatus having means for determining background radiation

International Nuclear Information System (INIS)

Randall, R.R.

1979-01-01

A neutron generator in a well logging instrument is periodically pulsed and has an off period between pulses of 1000 microseconds. A neutron detector is gated on at intervals of 400 to 500, 550 to 650, and 700 to 800 microseconds, respectively, following the termination of each burst of fast neutrons. Circuitry is provided for determining the background radiation by the equation: B = N 1 X N 3 - N 2 2 /N 1 + N 3 - 2N 2 where B is the background, and N 1 , N 2 and N 3 are the counts observed during the three gates, respectively. Circuitry is also provided for determining the macroscopic absorption (Σ) from the equation: Σ = 1/VΔt Log [N 1 - B/N 2 - B] where V is the velocity of thermal neutrons, being a constant and Δt represents an increment of time

Excitation methods for energy dispersive analysis

International Nuclear Information System (INIS)

Jaklevic, J.M.

1976-01-01

The rapid development in recent years of energy dispersive x-ray fluorescence analysis has been based primarily on improvements in semiconductor detector x-ray spectrometers. However, the whole analysis system performance is critically dependent on the availability of optimum methods of excitation for the characteristic x rays in specimens. A number of analysis facilities based on various methods of excitation have been developed over the past few years. A discussion is given of the features of various excitation methods including charged particles, monochromatic photons, and broad-energy band photons. The effects of the excitation method on background and sensitivity are discussed from both theoretical and experimental viewpoints. Recent developments such as pulsed excitation and polarized photons are also discussed

A nuclear radiation multi-parameter measurement system based on pulse-shape sampling

International Nuclear Information System (INIS)

Qiu Xiaolin; Fang Guoming; Xu Peng; Di Yuming

2007-01-01

In this paper, A nuclear radiation multi-parameter measurement system based on pulse-shape sampling is introduced, including the system's characteristics, composition, operating principle, experiment data and analysis. Compared with conventional nuclear measuring apparatus, it has some remarkable advantages such as the synchronous detection using multi-parameter measurement in the same measurement platform and the general analysis of signal data by user-defined program. (authors)

The doppler frequency shift caused by the inhomogeneities of a medium induced by pulses of intense laser radiation

Science.gov (United States)

Rozanov, N. N.; Kiselev, Al. S.; Kiselev, An. S.

2008-08-01

Self-reflection of pulses of intense laser radiation from an inhomogeneity induced by them in a medium with fast optical nonlinearity is analyzed. The reflected radiation is characterized by a considerable Doppler shift and by a signal magnitude that is sufficient for experimental detection.

Enhancement of deposition rate at cryogenic temperature in synchrotron radiation excited deposition of silicon film

International Nuclear Information System (INIS)

Nara, Yasuo; Sugita, Yoshihiro; Ito, Takashi; Kato, Hiroo; Tanaka, Ken-ichiro

1989-01-01

The authors have investigated the synchrotron radiation excited deposition of silicon films on the SiO 2 substrate by using SiH 4 /He mixture gas at BL-12C at Photon Factory. They used VUV light from the multilayer mirror with the center photon energy from 97 to 123eV, which effectively excites L-core electrons of silicon. Substrate temperature was widely varied from -178 degree C to 500 degree C. At -178 degree C, the deposition rate was as high as 400nm/200mAHr (normalized at the storage ring current at 200mA). As increasing the substrate temperature, the deposition rate was drastically decreased. The number of deposited silicon atoms is estimated to be 4 to 50% of incident photons, while the number of photo generated species in the gas phase within the mean free path from the surface is calculated as few as about 10 -3 of incident photons. These experimental results show that the deposition reaction is governed by the dissociation of surface adsorbates by the synchrotron radiation

On excitation and radiation of detector moving in vacuum with acceleration or moving rectilinearly with superluminal velocity in a medium

International Nuclear Information System (INIS)

Ginzburg, V.L.; Frolov, V.P.

1986-01-01

The problem of excitation of a detector moving in vacuum with constant acceleration is being discussed in recent years. It is noted in the paper that this excitation and radiation associated with it are similar to those taking place in the range of anomalous Doppler effect occurring during motion of the detector with constant superluminal velocity in medium

Lifetime measurements of highly excited Rydberg states of strontium. Pt. 1

International Nuclear Information System (INIS)

Kunze, S.; Hohmann, R.; Kluge, H.J.; Lantzsch, J.; Monz, L.; Stenner, J.; Stratmann, K.; Wendt, K.; Zimmer, K.

1993-01-01

Lifetimes of Rydberg states of triplet-series 5s ns 3 S 1 with n=19-23, 35 and 5s nd 3 D 3 with n=18-20, 23-28 in the spectrum of neutral strontium have been determined. Observation of the exponential decay after excitation by a pulsed laser in a fast atomic beam and subsequent state-selective field ionization was employed. The lifetimes of the states of the 3 S 1 -series show the expected n* 3 dependence on the effective principal quantum number, while the 3 D 3 -series is disturbed by configuration mixing. Furthermore, state re-populations induced by black-body radiation have been observed. (orig.)

Excitation and ionization of hydrogen and helium atoms by femtosecond laser pulses: theoretical approach by Coulomb-Volkov states; Excitation et ionisation des atomes d'hydrogene et d'helium par des impulsions laser femtosecondes: approche theorique par des etats de Coulomb-Volkov

Energy Technology Data Exchange (ETDEWEB)

Guichard, R

2007-12-15

We present a theoretical approach using Coulomb-Volkov states that appears useful for the study of atomic multi-photonic processes induced by intense XUV femtosecond laser pulses. It predicts hydrogen ionization spectra when it is irradiated by laser pulses in perturbations conditions. Three ways have been investigated. Extension to strong fields when {Dirac_h}{omega} > I{sub p}: it requires to include the hydrogen ground state population, introducing it in standard Coulomb-Volkov amplitude leads to saturated multi-photonic ionization. Extension to multi-photonic transitions with {Dirac_h}{omega} < I{sub p}: new quantum paths are open by the possibility to excite the lower hydrogen bound states. Multiphoton excitation of these states is investigated using a Coulomb-Volkov approach. Extension to helium: two-photon double ionization study shows the influence of electronic correlations in both ground and final state. Huge quantity of information such as angular and energetic distributions as well as total cross sections is available. (author)

Dynamics of laser-induced channel formation in water and influence of pulse duration on the ablation of biotissue under water with pulsed erbium-laser radiation

Science.gov (United States)

Ith, M.; Pratisto, H.; Altermatt, H. J.; Frenz, M.; Weber, H. P.

1994-12-01

The ability to use fiber-delivered erbium-laser radiation for non-contact arthroscopic meniscectomy in a liquid environment was studied. The laser radiation is transmitted through a water-vapor channel created by the leading part of the laser pulse. The dynamics of the channel formation around a submerged fiber tip was investigated with time-resolved flash photography. Strong pressure transients with amplitudes up to a few hundreds of bars measured with a needle hydrophone were found to accompany the channel formation process. Additional pressure transients in the range of kbars were observed after the laser pulse associated with the collapse of the vapor channel. Transmission measurements revealed that the duration the laser-induced channel stays open, and therefore the energy transmittable through it, is substantially determined by the laser pulse duration. The optimum pulse duration was found to be in the range between 250 and 350 µS. This was confirmed by histological evaluations of the laser incisions in meniscus: Increasing the pulse duration from 300 to 800 µs leads to a decrease in the crater depth from 1600 to 300 µm. A comparison of the histological examination after laser treatment through air and through water gave information on the influence of the vapor channel on the ablation efficiency, the cutting quality and the induced thermal damage in the adjacent tissue. The study shows that the erbium laser combined with an adequate fiber delivery system represents an effective surgical instrument liable to become increasingly accepted in orthopedic surgery.

Technical specifications manual for the MARK-1 pulsed ionizing radiation detection system. Volume 1

Energy Technology Data Exchange (ETDEWEB)

Lawrence, R.S.; Harker, Y.D.; Jones, J.L.; Hoggan, J.M.

1993-03-01

The MARK-1 detection system was developed by the Idaho National Engineering Laboratory for the US Department of Energy Office of Arms Control and Nonproliferation. The completely portable system was designed for the detection and analysis of intense photon emissions from pulsed ionizing radiation sources. This manual presents the technical design specifications for the MARK-1 detection system and was written primarily to assist the support or service technician in the service, calibration, and repair of the system. The manual presents the general detection system theory, the MARK-1 component design specifications, the acquisition and control software, the data processing sequence, and the system calibration procedure. A second manual entitled: Volume 2: Operations Manual for the MARK-1 Pulsed Ionizing Radiation Detection System (USDOE Report WINCO-1108, September 1992) provides a general operational description of the MARK-1 detection system. The Operations Manual was written primarily to assist the field operator in system operations and analysis of the data.

Spectral tuning via multi-phonon-assisted stokes and anti-stokes excitations in LaF{sub 3}: Tm{sup 3+} nanoparticles

Energy Technology Data Exchange (ETDEWEB)

Gao, Dangli, E-mail: gaodangli@163.com [School of Materials & Mineral Resources, Xi' an University of Architecture and Technology, Xi' an, Shaanxi 710055 (China); College of Science, Xi' an University of Architecture and Technology, Xi' an, Shaanxi 710055 (China); Shaanxi Key Laboratory of Nano Materials and Technology, Xi' an, Shaanxi 710055 (China); Tian, Dongping, E-mail: dptian@xauat.edu.cn [School of Materials & Mineral Resources, Xi' an University of Architecture and Technology, Xi' an, Shaanxi 710055 (China); College of Science, Xi' an University of Architecture and Technology, Xi' an, Shaanxi 710055 (China); Chong, Bo; Li, Long [College of Science, Xi' an University of Architecture and Technology, Xi' an, Shaanxi 710055 (China); Zhang, Xiangyu [College of Science, Chang' an University, Xi' an, Shaanxi 710064 (China)

2016-09-05

We present a facile and highly effective method to tailor upconversion (UC) emission from LaF{sub 3}: Tm{sup 3+} nanoparticles (NPs) by adjusting ambient temperature from 20 K to 400 K accompanied with the pulse laser excitation. Spectral tuning mechanism controlled by ambient temperature at pulse laser excitation is revealed, and a mechanism based on the modification on multi-phonon relaxation rates for the rapid population of intermediate level {sup 3}H{sub 4} and multi-phonon-assisted excited state absorption is proposed. Based on multi-phonon relaxation theory and time-resolved photoluminescence studies, it is reasonable that UC luminescence under short-pulse laser excitation mainly originates from the ions at/near the surface of NPs. These exciting findings in ambient temperature accompanied with the short-pulse excitation dependent UC selectivity offer a general approach to tailoring lanthanide related UC emissions, which will benefit multicolor displays and imaging. - Graphical abstract: An effective method to tailor upconversion from LaF{sub 3}: Tm{sup 3+} nanoparticles by adjusting ambient temperature accompanied with the short-pulse laser excitation is presented and the spectral tuning mechanism based the modification on multi-phonon relaxation rate and multi-phonon-assisted excited state absorption is also revealed. - Highlights: • The luminescence switching is controlled by temperature and pulse duration. • The mechanism based on the multi-phonon-assisted excitations is proposed. • Blue luminescence under short-pulse excitation originates from the surface ions. • Temperature has a big effect on luminescence color output.

Measured pulse width of sonoluminescence flashes in the form of resonance radiation

Science.gov (United States)

Giri, Asis; Arakeri, Vijay H.

1998-09-01

Recent studies have shown that the measured flash widths from single and multibubble sonoluminescence are in subnanosecond or even picosecond regime. Here, we provide conclusive evidence for the existence of nanosecond multibubble sonoluminescence. This has become possible by our ability to find a medium from which exclusive sodium D line resonance radiation as a form of sonoluminescence is possible. The measured flash width of this emission is found to be in the range of tens of nanoseconds and is sensitively dependent on experimental parameters. Our finding is important since all the earlier pulse width measurements have been limited to emission with the physical source or species responsible for observed optical radiation not being clearly identified. We propose that the presently observed resonance radiation is from ``soft'' bubble collapse as analyzed by V. Kamath et al. [J. Acoust. Soc. Am. 94, 248 (1993)].

Generation of Femtosecond Electron and Photon Pulses

CERN Document Server

Thongbai, Chitrlada; Kangrang, Nopadol; Kusoljariyakul, Keerati; Rhodes, Michael W; Rimjaem, Sakhorn; Saisut, Jatuporn; Vilaithong, Thiraphat; Wichaisirimongkol, Pathom; Wiedemann, Helmut

2005-01-01

Femtosecond electron and photon pulses become a tool of interesting important to study dynamics at molecular or atomic levels. Such short pulses can be generated from a system consisting of an RF-gun with a thermionic cathode, an alpha magnet as a magnetic bunch compressor, and a linear accelerator. The femtosecond electron pulses can be used directly or used as sources to produce electromagnetic radiation of equally short pulses by choosing certain kind of radiation pruduction processes. At the Fast Neutron Research Facility (Thailand), we are especially interested in production of radiation in Far-infrared and X-ray regime. In the far-infrared wavelengths which are longer than the femtosecond pulse length, the radiation is emitted coherently producing intense radiation. In the X-ray regime, development of femtosecond X-ray source is crucial for application in ultrafast science.

Synchrotron radiation induced TXRF of low Z elements on Si wafer surfaces at SSRL-comparison of excitation geometries and condition

International Nuclear Information System (INIS)

Streli, C.; Wobrauschek, P.; Kregsamer, P.; Pepponi, G.; Pianetta, P.; Pahlke, S.; Fabry, L.

2000-01-01

The determination of low Z elements, like Na and Al at ultra trace levels on Si wafer surfaces is demanded by semiconductor industry. SR-TXRF is a promising method to fulfill the task, if a special energy dispersive detector with an ultra thin window is used. Synchrotron radiation is the ideal suited excitation source for TXRF of low Z elements due to its intensive, natural collimated and linear polarized radiation with wide spectral range down to low energies even below 1 keV. TXRF offers some advantages for wafer surface analysis like nondestructive investigation and mapping capability. Experiments have been performed at SSRL beamline 3-4, a bending magnet beamline using white (<3 keV) and monochromatic radiation, as well as on beamline 3-3, using a crystal monochromator as well as a multilayer monochromator. A comparison of excitation detection geometries was performed, using a sidelooking detector with vertical positioned wafer as well as a downlooking detector with a horizontally arranged wafer. The advantages and disadvantages of the various geometries and excitation conditions are presented and the results compared. Detection limits are in the 100 fg range for Na, determined with droplet samples on Si wafer surfaces. (author)

Computer simulation of the spatial distribution of optical radiation arising from knocked-out excited particles

International Nuclear Information System (INIS)

Gokov, S.P.; Gritsyna, V.V.; Koval', A.G.; Kovtunenko, Yu.I.; Shevchenko, D.I.

2004-01-01

The new approach for the explanation of the spatial distribution of the optical radiation arising from knocked-out excited particles is given. Calculated and experimental data for Al (λ=396.1 nm) and Mg (λ=383.8 nm) knocked-out by Ar + (20 keV) beam from MgAl 2 O 4 surface are compared [ru

Using narrowband excitation to confirm that the S∗ state in carotenoids is not a vibrationally-excited ground state species

Science.gov (United States)

Jailaubekov, Askat E.; Song, Sang-Hun; Vengris, Mikas; Cogdell, Richard J.; Larsen, Delmar S.

2010-02-01

The hypothesis that S∗ is a vibrationally-excited ground-state population is tested and discarded for two carotenoid samples: β-carotene in solution and rhodopin glucoside embedded in the light harvesting 2 protein from Rhodopseudomonas acidophila. By demonstrating that the transient absorption signals measured in both systems that are induced by broadband (1000 cm -1) and narrowband (50 cm -1) excitation pulses are near identical and hence bandwidth independent, the impulsive stimulated Raman scattering mechanism proposed as the primary source for S∗ generation is discarded. To support this conclusion, previously published multi-pulse pump-dump-probe signals [17] are revisited to discard secondary mechanisms for S∗ formation.

Irradiation of cells by single and double pulses of high intensity radiation: oxygen sensitization and diffusion kinetics

International Nuclear Information System (INIS)

Epp, E.R.; Ling, C.C.; Weiss, H.

1976-01-01

This paper discusses advances made on both experimental and theoretical approaches involving single and double pulses of high intensity ionizing radiation delivered to cultured bacterial and mammalian cells where the effect of oxygen is concerned. Information gained on the lifetime of oxygen-sensitive species suspected to be produced in critical molecules in irradiated cells and perhaps intimately related to the still unknown mechanisms of oxygen sensitization is described. The diffusion characteristics of oxygen at the cellular level obtained from experimental data are discussed. Current knowledge on intracellular radiolytic oxygen depletion is also presented. Future work on the use of high intensity pulsed radiation as a tool in cellular radiobiological research is outlined. It is expected that obtaining knowledge of the time available for damaged molecules to enter into chemical reactions may lead to insights into the mechanisms of radiation injury in cells, such as those involved in the oxygen effect. (Auth.)

Laser breakdown with millijoule trains of picosecond pulses transmitted through a hollow-core photonic-crystal fibre

CERN Document Server

Konorov, S O; Kolevatova, O A; Beloglasov, V I; Skibina, N B; Shcherbakov, A V; Wintner, E; Zheltikov, A M

2003-01-01

Sequences of picosecond pulses with a total energy in the pulse train of about 1 mJ are transmitted through a hollow-core photonic-crystal fibre with a core diameter of approximately 14 mu m. The fluence of laser radiation coupled into the core of the fibre under these conditions exceeds the breakdown threshold of fused silica by nearly an order of magnitude. The laser beam coming out of the fibre is then focused to produce a breakdown on a solid surface. Parameters of laser radiation were chosen in such a way as to avoid effects related to the excitation of higher order waveguide modes and ionization of the gas filling the fibre in order to provide the possibility to focus the output beam into a spot with a minimum diameter, thus ensuring the maximum spatial resolution and the maximum power density in the focal spot.

Electromagnetic Fields, Pulsed Radiofrequency Radiation, and Epigenetics: How Wireless Technologies May Affect Childhood Development

Science.gov (United States)

Sage, Cindy; Burgio, Ernesto

2018-01-01

Mobile phones and other wireless devices that produce electromagnetic fields (EMF) and pulsed radiofrequency radiation (RFR) are widely documented to cause potentially harmful health impacts that can be detrimental to young people. New epigenetic studies are profiled in this review to account for some neurodevelopmental and neurobehavioral changes…

Radiation dose reduction in CT-guided sacroiliac joint injections to levels of pulsed fluoroscopy: a comparative study with technical considerations

Directory of Open Access Journals (Sweden)

Artner J

2012-08-01

Full Text Available Juraj Artner, Balkan Cakir, Heiko Reichel, Friederike LattigDepartment of Orthopaedic Surgery, University of Ulm, RKU, GermanyBackground: The sacroiliac (SI joint is frequently the primary source of low back pain. Over the past decades, a number of different SI injection techniques have been used in its diagnosis and therapy. Despite the concerns regarding exposure to radiation, image-guided injection techniques are the preferred method to achieve safe and precise intra-articular needle placement. The following study presents a comparison of radiation doses, calculated for fluoroscopy and CT-guided SI joint injections in standard and low-dose protocol and presents the technical possibility of CT-guidance with maximum radiation dose reduction to levels of fluoroscopic-guidance for a precise intra-articular injection technique.Objective: To evaluate the possibility of dose reduction in CT-guided sacroiliac joint injections to pulsed-fluoroscopy-guidance levels and to compare the doses of pulsed-fluoroscopy-, CT-guidance, and low-dose CT-guidance for intra-articular SI joint injections.Study design: Comparative study with technical considerations.Methods: A total of 30 CT-guided intra-articular SI joint injections were performed in January 2012 in a developed low-dose mode and the radiation doses were calculated. They were compared to 30 pulsed-fluoroscopy-guided SI joint injections, which were performed in the month before, and to five injections, performed in standard CT-guided biopsy mode for spinal interventions. The statistical significance was calculated with the SPSS software using the Mann–Whitney U-Test. Technical details and anatomical considerations were provided.Results: A significant dose reduction of average 94.01% was achieved using the low-dose protocol for CT-guided SI joint injections. The radiation dose could be approximated to pulsed-fluoroscopy-guidance levels.Conclusion: Radiation dose of CT-guided SI joint injections can be

Digital pulse processing techniques for high resolution amplitude measurement of radiation detector

International Nuclear Information System (INIS)

Singhai, P.; Roy, A.; Dhara, P.; Chatterjee, S.

2012-01-01

The digital pulse processing techniques for high resolution amplitude measurement of radiation detector pulse is an effective replacement of expensive and bulky analog processing as the digital domain offers higher channel density and at the same time it is cheaper. We have demonstrated a prototype digital setup with highspeed sampling ADC with sampling frequency of 80-125 MHz followed by series of IIR filters for pulse shaping in a trigger-less acquisition mode. The IIR filters, peak detection algorithm and the data write-out logic was written on VHDL and implemented on FPGA. We used CAMAC as the read out platform. In conjunction with the full hardware implementation we also used a mixed platform with VME digitizer card with raw-sample read out using C code. The rationale behind this mixed platform is to test out various filter algorithms quickly on C and also to benchmark the performance of the chip level ADCs against the standard commercial digitizer in terms of noise or resolution. The paper describes implementation of both the methods with performance obtained in both the methods. (author)

Absolute carrier phase effects in the two-color excitation of dipolar molecules

International Nuclear Information System (INIS)

Brown, Alex; Meath, W.J.; Kondo, A.E.

2002-01-01

The pump-probe excitation of a two-level dipolar (d≠0) molecule, where the pump frequency is tuned to the energy level separation while the probe frequency is extremely small, is examined theoretically as an example of absolute phase control of excitation processes. The state populations depend on the probe field's absolute carrier phase but are independent of the pump field's absolute carrier phase. Interestingly, the absolute phase effects occur for pulse durations much longer and field intensities much weaker than those required to see such effects in single pulse excitation

Photoinduced dynamics of a cyanine dye: parallel pathways of non-radiative deactivation involving multiple excited-state twisted transients.

Science.gov (United States)

Upadhyayula, Srigokul; Nuñez, Vicente; Espinoza, Eli M; Larsen, Jillian M; Bao, Duoduo; Shi, Dewen; Mac, Jenny T; Anvari, Bahman; Vullev, Valentine I

2015-04-01

Cyanine dyes are broadly used for fluorescence imaging and other photonic applications. 3,3'-Diethylthiacyanine (THIA) is a cyanine dye composed of two identical aromatic heterocyclic moieties linked with a single methine, -CH 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 1111111111111111111111111111111111 1111111111111111111111111111111111 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 1111111111111111111111111111111111 1111111111111111111111111111111111 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 0000000000000000000000000000000000 . The torsional degrees of freedom around the methine bonds provide routes for non-radiative decay, responsible for the inherently low fluorescence quantum yields. Using transient absorption spectroscopy, we determined that upon photoexcitation, the excited state relaxes along two parallel pathways producing three excited-state transients that undergo internal conversion to the ground state. The media viscosity impedes the molecular modes of ring rotation and preferentially affects one of the pathways of non-radiative decay, exerting a dominant effect on the emission

Radiative and non-radiative relaxation of excitons in strain-compensated quantum dots

International Nuclear Information System (INIS)

Kujiraoka, M.; Ishi-Hayase, J.; Akahane, K.; Yamamoto, Y.; Ema, K.; Sasaki, M.

2008-01-01

We have investigated the population dynamics of excitons in strain-compensated InAs quantum dots (QDs) using a pump-probe technique under resonant excitation. Precise control of polarization directions of incident pulses enabled us to selectively estimate population lifetimes for two orthogonally polarized exciton ground states according to polarization selection rules. Measured decay times of the probe transmissions were highly dependent on the polarization directions of the exciton states. We found that the ratio of the decay times for the orthogonally polarized states is in quantitative agreement with the ratio of square of the transition dipole moments. This indicates that radiative recombination processes have a dominant effect on the population dynamics and that non-radiative and spin relaxations are negligible in our QDs. As a result, we can estimate the radiative lifetimes to be 1.0±0.1 and 1.7±0.2 ns for orthogonally polarized exciton ground states

Pulsed air-core deflector-magnet design parameters

International Nuclear Information System (INIS)

Jason, A.J.; Cooper, R.K.; Liebman, A.D.; Blind, B.; Koelle, A.R.

1983-01-01

The response of air-core magnets to pulsed excitation is dependent on the pulse frequency spectrum because of fields produced by induced currents in the magnet structure. We discuss this phenomenon quantitatively in terms of magnet performance optimization

Towards diffractive imaging with single pulses of FEL radiation. Dynamics within irradiatied samples and their influence on the analysis of imaging data

Energy Technology Data Exchange (ETDEWEB)

Wang, Fenglin

2010-08-15

3D single particle coherent diffraction imaging (CDI) of bioparticles (such as proteins, macromolecules and viruses) is one of the main possible applications of the new generation of light sources: free-electron lasers (FELs), which are now available at FLASH (Hamburg, Germany) and LCLS (Stanford, U.S.A.). The extremely bright and ultrashort FEL pulses potentially enable CDI to achieve high resolution down to subnanometer length scale. However, intense FEL pulses cause serious radiation damage in bioparticles, even during single shots, which may set the resolution limits for CDI with FELs. Currently, since the signal-to-noise ratio is very low for small biological particles, direct experimental study of radiation damage in the single particle imaging is fairly difficult. Single atomic (noble gas) clusters become good objects to reveal effects of radiation damage processes on CDI with FEL radiation. This thesis studies three aspects of the radiation damage problem, which are treated in three independent chapters: (1) Molecular Dynamics simulations to quantitively describe radiation damage processes within irradiated atomic clusters during single pulses; (2) reconstruction analysis of single-shot CDI diffraction patterns of atomic clusters, which may potentially help to understand the radiation damage occurring in biological samples; and (3) testing the effects of coating water layers in CDI, which is supposed to minimize the radiation damage in irradiated bioparticles. (orig.)

LIME - a flexible, non-LTE line excitation and radiation transfer method for millimeter and far-infrared wavelengths

DEFF Research Database (Denmark)

Brinch, Christian; Hogerheijde, Michiel

2010-01-01

We present a new code for solving the molecular and atomic excitation and radiation transfer problem in a molecular gas and predicting emergent spectra. This code works in arbitrary three dimensional geometry using unstructured Delaunay latices for the transport of photons. Various physical model...

Demonstration of radiation pulse shaping with nested-tungsten-wire-array pinches for high-yield inertial confinement fusion.

Science.gov (United States)

Cuneo, M E; Vesey, R A; Sinars, D B; Chittenden, J P; Waisman, E M; Lemke, R W; Lebedev, S V; Bliss, D E; Stygar, W A; Porter, J L; Schroen, D G; Mazarakis, M G; Chandler, G A; Mehlhorn, T A

2005-10-28

Nested wire-array pinches are shown to generate soft x-ray radiation pulse shapes required for three-shock isentropic compression and hot-spot ignition of high-yield inertial confinement fusion capsules. We demonstrate a reproducible and tunable foot pulse (first shock) produced by interaction of the outer and inner arrays. A first-step pulse (second shock) is produced by inner array collision with a central CH2 foam target. Stagnation of the inner array at the axis produces the third shock. Capsules optimized for several of these shapes produce 290-900 MJ fusion yields in 1D simulations.

Study of the oncogenic expression in human fibroblast cells after exposure to very short pulsed laser radiations

International Nuclear Information System (INIS)

Dormont, D.; Freville, Th.; Raoul, H.; Courant, D.; Court, L.

1992-01-01

The aim of this study is to evaluate the capacity of a laser, delivering very short pulses in the near infrared spectrum with a high pulse ratio frequency, to induce genetic modification on biological tissues. The absence of dicentric among chromosomal aberrations on human lymphocytes suggests that a repetitive very short pulses irradiation has a relatively low capacity to induce genetic abnormalities. The studies of the radiation effects on the cellular growth and the oncogenic expression show that the modifications, induced at the cellular level, do not seem the origin of a cellular transformation and a possible mechanism of carcinogenesis. (author)

Measurement and analysis of the electric field radiation in pulsed power system of linear induction accelerator

International Nuclear Information System (INIS)

Cheng Qifeng; Ni Jianping; Meng Cui; Cheng Cheng; Liu Yinong; Li Jin

2009-01-01

The close of high voltage switch in pulsed power system of linear induction accelerator often radiates strong transient electric field, which may influence ambient sensitive electric equipment, signals and performance of other instruments, etc. By performing gridded measurement around the Marx generator, the general distribution law and basic characters of electric field radiation are summarized. The current signal of the discharge circuit is also measured, which demonstrates that the current and the radiated electric field both have a resonance frequency about 150 kHz, and contain much higher frequency components. (authors)

Use of synchrotron and laser radiations for present and future photoionization studies in excited atoms and ions

International Nuclear Information System (INIS)

Wuilleumier, F.J.

1984-01-01

The status of experiments in photoionization of atoms in excited states is reviewed, with emphasis given to synchrotron and laser photon sources. A technique for exciting the photoionization spectrum of Na atoms using the flux emitted from the bending magnetic of a storage ring is discussed in detail. Some problems in interpreting photoionization spectrum of Ba in the excited state, due to the presence of higher orders are considered. A design approach for a positron storage ring to produce coherent radiation in the VUV is described. It is shown that combined use of a CW dye laser and the positron storage ring will allow new progress to be made in photoionization studies of excited atoms. Some of the experiments to be carried out using the positron storage ring include: measurements of collisional ionization in rare earth metal atoms of low atomic density; photoionization measurements at lower laser powers, leading to an extension of the CW tunability range; and photoionization studies of multiply charged positive ions. 21 references

vuv fluorescence from selective high-order multiphoton excitation of N2

International Nuclear Information System (INIS)

Coffee, Ryan N.; Gibson, George N.

2004-01-01

Recent fluorescence studies suggest that ultrashort pulse laser excitation may be highly selective. Selective high-intensity laser excitation holds important consequences for the physics of multiphoton processes. To establish the extent of this selectivity, we performed a detailed comparative study of the vacuum ultraviolet fluorescence resulting from the interaction of N 2 and Ar with high-intensity infrared ultrashort laser pulses. Both N 2 and Ar reveal two classes of transitions, inner-valence ns ' l ' . From their pressure dependence, we associate each transition with either plasma or direct laser excitation. Furthermore, we qualitatively confirm such associations with the time dependence of the fluorescence signal. Remarkably, only N 2 presents evidence of direct laser excitation. This direct excitation produces ionic nitrogen fragments with inner-valence (2s) holes, two unidentified transitions, and one molecular transition, the N 2 + :X 2 Σ g + 2 Σ u + . We discuss these results in the light of a recently proposed model for multiphoton excitation

Generation of high-power terahertz radiation by femtosecond-terawatt lasers

International Nuclear Information System (INIS)

Nashima, Shigeki; Hosoda, Makoto; Daido, Hiroyuki

2007-01-01

We observed electromagnetic waves in the terahertz (THz) frequency range from a Ti foil excited by tabletop terawatt (T-cube) laser pulses. The radiation power was increased drastically with increasing its laser power. We also investigated the polarization characteristics of the sub-terahertz wave. It is found that the polarization of the radiated sub-terahertz waves was parallel to the incident beam plane, which is independent on the pump laser polarization. These results indicate transient electric field to the incident plane is generated by laser-plasma interaction, i.e., laser wake field and coherent plasma wave. (author)

Superharmonic imaging with chirp coded excitation: filtering spectrally overlapped harmonics.