Spin liquid in a single crystal of the frustrated diamond lattice antiferromagnet CoAl2O4
Zaharko, O.; Christensen, Niels Bech; Cervellino, A.
2011-01-01
We study the evidence for spin liquid in the frustrated diamond lattice antiferromagnet CoAl2O4 by means of single-crystal neutron scattering in zero and applied magnetic fields. The magnetically ordered phase appearing below T-N = 8 K remains nonconventional down to 1.5 K. The magnetic Bragg peaks...
Zaharko, O.; Cervellino, A.; Tsurkan, V.
2010-01-01
Using neutron powder diffraction and Monte Carlo simulations we show that a spin-liquid regime emerges at all compositions in the diamond-lattice antiferromagnets Co(Al1−xCox)2O4. This spin-liquid regime induced by frustration due to the second-neighbor exchange coupling J2 is gradually superseded...
Hirose, Yuhei; Oguchi, Akihide; Fukumoto, Yoshiyuki
2016-09-01
We study Heisenberg antiferromagnets on a diamond-like decorated square lattice perturbed by further neighbor couplings. The second-order effective Hamiltonian is calculated and the resultant Hamiltonian is found to be a square-lattice quantum-dimer model with a finite hopping amplitude and no repulsion, which suggests the stabilization of the plaquette phase. Our recipe for constructing quantum-dimer models can be adopted for other lattices and provides a route for the experimental realization of quantum-dimer models.
Hirose, Yuhei; Oguchi, Akihide; Fukumoto, Yoshiyuki
2017-01-01
We study the ground-state phase diagram of a Heisenberg model with spin S = 1/2 on a diamond-like-decorated square lattice. A diamond unit has two types of antiferromagnetic exchange interactions, and the ratio λ of the length of the diagonal bond to that of the other four edges determines the strength of frustration. It has been pointed out [https://doi.org/10.7566/JPSJ.85.033705" xlink:type="simple">J. Phys. Soc. Jpn 85, 033705 (2016)] that the so-called tetramer-dimer states, which are expected to be stabilized in an intermediate region of λc < λ < 2, are identical to the square-lattice dimer-covering states, which ignited renewed interest in high-dimensional diamond-like-decorated lattices. In order to determine the phase boundary λc, we employ the modified spin wave method to estimate the energy of the ferrimagnetic state and obtain λc = 0.974. Furthermore, our numerical diagonalization study suggests that other cluster states do not appear in the ground-state phase diagram.
Spin order and dynamics in the diamond-lattice Heisenberg antiferromagnets CuRh2O4 and CoRh2O4
Ge, L.; Flynn, J.; Paddison, J. A. M.; Stone, M. B.; Calder, S.; Subramanian, M. A.; Ramirez, A. P.; Mourigal, M.
2017-08-01
Antiferromagnetic insulators on a diamond lattice are candidate materials to host exotic magnetic phenomena ranging from spin-orbital entanglement to degenerate spiral ground states and topological paramagnetism. Compared to other three-dimensional networks of magnetic ions, such as the geometrically frustrated pyrochlore lattice, the investigation of diamond-lattice magnetism in real materials is less mature. In this work, we characterize the magnetic properties of model A -site spinels CoRh2O4 (cobalt rhodite) and CuRh2O4 (copper rhodite) by means of thermomagnetic and neutron-scattering measurements, and we perform group theory analysis, Rietveld refinement, mean-field theory, and spin-wave theory calculations to analyze the experimental results. Our investigation reveals that cubic CoRh2O4 is a canonical S =3 /2 diamond-lattice Heisenberg antiferromagnet with a nearest-neighbor exchange J =0.63 meV and a Néel ordered ground state below a temperature of 25 K. In tetragonally distorted CuRh2O4 , competing exchange interactions between up to third-nearest-neighbor spins lead to the development of an incommensurate spin helix at 24 K with a magnetic propagation vector km=(0 ,0 ,0.79 ) . Strong reduction of the ordered moment is observed for the S =1 /2 spins in CuRh2O4 and captured by our 1 /S corrections to the staggered magnetization. Our work identifies CoRh2O4 and CuRh2O4 as reference materials to guide future work searching for exotic quantum behavior in diamond-lattice antiferromagnets.
Antiferromagnetic Ising model on the swedenborgite lattice
Buhrandt, Stefan; Fritz, Lars
2014-01-01
Geometrical frustration in spin systems often results in a large number of degenerate ground states. In this work, we study the antiferromagnetic Ising model on the three-dimensional swedenborgite lattice, which is a specific stacking of kagome and triangular layers. The model contains two exchange
Lattice distortion in disordered antiferromagnetic XY models
Li Peng-Fei; Cao Hai-Jing
2012-01-01
The behavior of lattice distortion in spin 1/2 antiferromagnetic XY models with random magnetic modulation is investigated with the consideration of spin-phonon coupling in the adiabatic limit.It is found that lattice distortion relies on the strength of the random modulation.For strong or weak enough spin-phonon couplings,the average lattice distortion may decrease or increase as the random modulation is strengthened.This may be the result of competition between the random magnetic modulation and the spin-phonon coupling.
Antiferromagnetic noise correlations in optical lattices
Bruun, Niels Bohr International Academy, University of Copenhagen, DK-2100 Copenhagen Ø, Denmark, Georg Morten; Syljuåsen, F. T.; Pedersen, K. G. L.;
2009-01-01
We analyze how noise correlations probed by time-of-flight experiments reveal antiferromagnetic (AF) correlations of fermionic atoms in two-dimensional and three-dimensional optical lattices. Combining analytical and quantum Monte Carlo calculations using experimentally realistic parameters, we...... show that AF correlations can be detected for temperatures above and below the critical temperature for AF ordering. It is demonstrated that spin-resolved noise correlations yield important information about the spin ordering. Finally, we show how to extract the spin correlation length and the related...
Frustrated diamond-chain quantum XXZ Heisenberg antiferromagnet in a magnetic field
Richter, Johannes, E-mail: Johannes.Richter@Physik.Uni-Magdeburg.DE [Institut für theoretische Physik, Otto-von-Guericke-Universität Magdeburg, P.O. Box 4120, D-39016 Magdeburg (Germany); Krupnitska, Olesia [Institute for Condensed Matter Physics, National Academy of Sciences of Ukraine, 1 Svientsitskii Street, L' viv-11, 79011 (Ukraine); Krokhmalskii, Taras [Institute for Condensed Matter Physics, National Academy of Sciences of Ukraine, 1 Svientsitskii Street, L' viv-11, 79011 (Ukraine); Department for Theoretical Physics, Ivan Franko National University of L' viv, 12 Drahomanov Street, L' viv-5, 79005 (Ukraine); Derzhko, Oleg [Institut für theoretische Physik, Otto-von-Guericke-Universität Magdeburg, P.O. Box 4120, D-39016 Magdeburg (Germany); Institute for Condensed Matter Physics, National Academy of Sciences of Ukraine, 1 Svientsitskii Street, L' viv-11, 79011 (Ukraine); Department for Theoretical Physics, Ivan Franko National University of L' viv, 12 Drahomanov Street, L' viv-5, 79005 (Ukraine); Abdus Salam International Centre for Theoretical Physics, Strada Costiera 11, I-34151 Trieste (Italy)
2015-04-01
We consider the antiferromagnetic spin-1/2 XXZ Heisenberg model on a frustrated diamond-chain lattice in a z- or x-aligned external magnetic field. We use the strong-coupling approach to elaborate an effective description in the low-temperature strong-field regime. The obtained effective models are spin-1/2 XY chains which are exactly solvable through the Jordan–Wigner fermionization. We perform exact-diagonalization studies of the magnetization curves to test the quality of the effective description. The results may have relevance for the description of the azurite spin-chain compound.
Supersymmetry protected topological phases of isostatic lattices and kagome antiferromagnets
Lawler, Michael J.
2016-10-01
I generalize the theory of phonon topological band structures of isostatic lattices to frustrated antiferromagnets. I achieve this with a discovery of a many-body supersymmetry (SUSY) in the phonon problem of balls and springs and its connection to local constraints satisfied by ground states. The Witten index of the SUSY model demands the Maxwell-Calladine index of mechanical structures. "Spontaneous supersymmetry breaking" is identified as the need to gap all modes in the bulk to create the topological isostatic lattice state. Since ground states of magnetic systems also satisfy local constraint conditions (such as the vanishing of the total spin on a triangle), I identify a similar SUSY structure for many common models of antiferromagnets including the square, triangluar, kagome, pyrochlore nearest-neighbor antiferromagnets, and the J2=J1/2 square-lattice antiferromagnet. Remarkably, the kagome family of antiferromagnets is the analog of topological isostatic lattices among this collection of models. Thus, a solid-state realization of the theory of phonon topological band structure may be found in frustrated magnetic materials.
On diamond-free subposets of the Boolean lattice
Kramer, Lucas; Young, Michael
2012-01-01
The Boolean lattice of dimension two, also known as the diamond, consists of four distinct elements with the following property: $A\\subset B,C\\subset D$. A diamond-free family in the $n$-dimensional Boolean lattice is a subposet such that no four elements form a diamond. Note that elements $B$ and $C$ may or may not be related. There is a diamond-free family in the $n$-dimensional Boolean lattice of size $(2-o(1)){n\\choose\\lfloor n/2\\rfloor}$. In this paper, we prove that any diamond-free family in the $n$-dimensional Boolean lattice has size at most $(2.25+o(1)){n\\choose\\lfloor n/2\\rfloor}$. Furthermore, we show that the so-called Lubell function of a diamond-free family in the $n$-dimensional Boolean lattice is at most $2.25+o(1)$, which is asympotically best possible.
Correlations between Kondo clouds in nearly antiferromagnetic Kondo lattices
Kiselev, M.N. E-mail: kiselev@physik.uni-wuerzburg.de; Kikoin, K.A
2004-05-01
We discuss a novel fluctuational mechanism explaining the physics of nearly antiferromagnetic Kondo lattices (KL). The effective action for KL model is expressed in terms of Bose operators responsible for paramagnetic excitations and semi-bosonic fields describing the dynamic Kondo clouds created by conduction electrons around local spin. The gauge invariant resonance valence bond theory of interacting Kondo clouds describes the spin liquid with strong critical fluctuations imitating itinerant fluctuation magnetism of Moriya type.
Fractional excitations in the square-lattice quantum antiferromagnet
Dalla Piazza, B.; Mourigal, M.; Christensen, N. B.; Nilsen, G. J.; Tregenna-Piggott, P.; Perring, T. G.; Enderle, M.; McMorrow, D. F.; Ivanov, D. A.; Rønnow, H. M.
2015-01-01
Quantum magnets have occupied the fertile ground between many-body theory and low-temperature experiments on real materials since the early days of quantum mechanics. However, our understanding of even deceptively simple systems of interacting spin-1/2 particles is far from complete. The quantum square-lattice Heisenberg antiferromagnet, for example, exhibits a striking anomaly of hitherto unknown origin in its magnetic excitation spectrum. This quantum effect manifests itself for excitations propagating with the specific wavevector (π, 0). We use polarized neutron spectroscopy to fully characterize the magnetic fluctuations in the metal-organic compound Cu(DCOO)2.4D2O, a known realization of the quantum square-lattice Heisenberg antiferromagnet model. Our experiments reveal an isotropic excitation continuum at the anomaly, which we analyse theoretically using Gutzwiller-projected trial wavefunctions. The excitation continuum is accounted for by the existence of spatially extended pairs of fractional S = 1/2 quasiparticles, 2D analogues of 1D spinons. Away from the anomalous wavevector, these fractional excitations are bound and form conventional magnons. Our results establish the existence of fractional quasiparticles in the high-energy spectrum of a quasi-two-dimensional antiferromagnet, even in the absence of frustration.
Spin-Lattice-Coupled Order in Heisenberg Antiferromagnets on the Pyrochlore Lattice
Aoyama, Kazushi; Kawamura, Hikaru
2016-06-01
Effects of local lattice distortions on the spin ordering are investigated for the antiferromagnetic classical Heisenberg model on the pyrochlore lattice. It is found by Monte Carlo simulations that the spin-lattice coupling (SLC) originating from site phonons induces a first-order transition into two different types of collinear magnetic ordered states. The state realized at the stronger SLC is cubic symmetric characterized by the magnetic (1/2 ,1/2 ,1/2 ) Bragg peaks, while that at the weaker SLC is tetragonal symmetric characterized by the (1,1,0) ones, each accompanied by the commensurate local lattice distortions. Experimental implications to chromium spinels are discussed.
Spin-Lattice-Coupled Order in Heisenberg Antiferromagnets on the Pyrochlore Lattice.
Aoyama, Kazushi; Kawamura, Hikaru
2016-06-24
Effects of local lattice distortions on the spin ordering are investigated for the antiferromagnetic classical Heisenberg model on the pyrochlore lattice. It is found by Monte Carlo simulations that the spin-lattice coupling (SLC) originating from site phonons induces a first-order transition into two different types of collinear magnetic ordered states. The state realized at the stronger SLC is cubic symmetric characterized by the magnetic (1/2,1/2,1/2) Bragg peaks, while that at the weaker SLC is tetragonal symmetric characterized by the (1,1,0) ones, each accompanied by the commensurate local lattice distortions. Experimental implications to chromium spinels are discussed.
Ferromagnetic and antiferromagnetic order in bacterial vortex lattices
Wioland, Hugo; Woodhouse, Francis G.; Dunkel, Jörn; Goldstein, Raymond E.; Goldstein Lab Team
2013-11-01
In conventional electronic materials, spins can organize into ordered phases that give rise to ferromagnetic or antiferromagnetic behavior. Here, we report similar observations in a completely different system: a suspension of swimming bacteria. When a dense Bacillus subtilis suspension is confined to a small circular chamber, it can spontaneously form a stable vortex (``spin'') state that can persist for several minutes. By coupling up to 100 such chambers in microfluidic devices, we are able to realize bacterial spin lattices of different geometries. Depending on that geometry and the effective coupling strength between neighboring vortices, we observe the formation of stable ``antiferromagnetic'' and ``ferromagnetic'' bacterial vortex states, that appear to be controlled by the subtle competition between bacterial boundary layer flows and bulk dynamics.
The Heisenberg antiferromagnet on the square-kagomé lattice
J. Richter
2009-01-01
Full Text Available We discuss the ground state, the low-lying excitations as well as high-field thermodynamics of the Heisenberg antiferromagnet on the two-dimensional square-kagomé lattice. This magnetic system belongs to the class of highly frustrated spin systems with an infinite non-trivial degeneracy of the classical ground state as it is also known for the Heisenberg antiferromagnet on the kagomé and on the star lattice. The quantum ground state of the spin-half system is a quantum paramagnet with a finite spin gap and with a large number of non-magnetic excitations within this gap. We also discuss the magnetization versus field curve that shows a plateaux as well as a macroscopic magnetization jump to saturation due to independent localized magnon states. These localized states are highly degenerate and lead to interesting features in the low-temperature thermodynamics at high magnetic fields such as an additional low-temperature peak in the specific heat and an enhanced magnetocaloric effect.
Mechanical Properties of Laser-Sintered-Nylon Diamond Lattices
Neff, Clayton
Additive manufacturing offers a manufacturing technique to produce complex geometry prototypes at a rapid pace and low cost. These advantages advocate additive manufacturing for the design and production of cellular structures. Cellular structures are interesting because they contain a large amount of porosity (void space of air) to manifest a lightweight structure. Designs of cellular structures generate a periodic pattern; often of complex geometry, called a lattice. There has been a significant amount of research to maximize specific stiffness of lattice structures but little to evaluate low-stiffness lattices. Low-stiffness structures benefit energy absorbance through bending of the lattice. This research seeks to assess diamond lattices as low stiffness, bending structures. The research involves PA2200 (Nylon 12) laser sintered diamond lattices with experimental compression testing and direct FEA model comparison. A correction factor is applied for a design offset of laser sintered lattices. Once applied, the experimental and FEA data agree in validating the diamond lattice as a bending-dominated structure. Diamond lattices show a 4th order relationship between stiffness and parameters of thickness and unit cell length. For density, stiffness maintains a 2nd order relationship, as predicted by bending dominated structures. The resulting stiffness can be tuned over a stiffness range of four orders of magnitude. Further research shows the results for modifying the diamond lattice and scaling stiffness and density using other materials (like metals) to expand the range of stiffness and compare diamond lattices on material property charts. Lastly, the effective Poisson's ratio varies from 0.5 to 0.4 depending on the (t/L) ratio.
Three-sublattice skyrmion crystal in the antiferromagnetic triangular lattice
Rosales, H. D.; Cabra, D. C.; Pujol, Pierre
2015-12-01
The frustrated classical antiferromagnetic Heisenberg model with Dzyaloshinskii-Moriya (DM) interactions on the triangular lattice is studied under a magnetic field by means of semiclassical calculations and large-scale Monte Carlo simulations. We show that even a small DM interaction induces the formation of an antiferromagnetic skyrmion crystal (AF-SkX) state. Unlike what is observed in ferromagnetic materials, we show that the AF-SkX state consists of three interpenetrating skyrmion crystals (one by sublattice), and most importantly, the AF-SkX state seems to survive in the limit of zero temperature. To characterize the phase diagram we compute the average of the topological order parameter which can be associated with the number of topological charges or skyrmions. As the magnetic field increases this parameter presents a clear jump, indicating a discontinuous transition from a spiral phase into the AF-SkX phase, where multiple Bragg peaks coexist in the spin structure factor. For higher fields, a second (probably continuous) transition occurs into a featureless paramagnetic phase.
Quantum Phase Transitions in Anti-ferromagnetic Planar Cubic Lattices
Wellard, C J; Wellard, Cameron; Orus, Roman
2004-01-01
Motivated by its relation to an NP-hard problem we analyze the ground state properties of anti-ferromagnetic Ising-spin networks in planar cubic lattices under the action of homogeneous transverse and longitudinal magnetic fields. We consider different instances of the cubic geometry and find a set of quantum phase transitions for each one of the systems, which we characterize by means of entanglement behavior and majorization theory. Entanglement scaling at the critical region is in agreement with results arising from conformal symmetry, therefore even the simplest planar systems can display very large amounts of quantum correlation. No conclusion can be made as to the scaling behavior of the minimum energy gap, with the data allowing equally good fits to exponential and power law decays. Analysis of entanglement and especially of majorization instead of the energy spectrum proves to be a good way of detecting quantum phase transitions in highly frustrated configurations.
High magnetic field magnetization of a new triangular lattice antiferromagnet
Zhou, H. D. [Univ. of Tennessee, Knoxville, TN (United States); Los Alamos National Lab. (LANL), Los Alamos, NM (United States). National High Magnetic Field Lab. (MagLab); Stritzinger, Laurel Elaine Winter [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Harrison, Neil [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
2017-03-23
In CsV(MoO_{4})_{2}, the magnetic V^{3+} ions with octahedral oxygen-coordination form a geometrically frustrated triangular lattice. So fare, there is no magnetic properties reported on it. Recently, we successfully grew single crystals of CsV(MoO_{4})_{2} by using flux method. The susceptibility shows a sharp drop around 24 K, representing a long range magnetic ordering. To understand the physical properties of this new triangular lattice antiferromagnet (TLAF), we pursued high field magnetization measurements to answer two questions: (i) what is the saturation field, which will be very useful to calculate the exchange interaction of the system? (ii) Will it exhibit spin state transition, such as the up up down phase with 1/3-saturation moment as other TLAFs? Recently, we performed VSM measurements in Cell 8, Tallahassee, NHMFL, the results show that the magnetization reaches 0.38 MuB at 34 T, which is just 19% of the full moment of 2 MuB for V^{3+} (3d^{2}) ions. Apparently we need higher field to reach 1/3 value or full moment.
Evaluation of Watson-like integrals for a hyper bcc antiferromagnetic lattice
Radošević, S. M.; Pantić, M. R.; Kapor, D. V.; Pavkov-Hrvojević, M. V.; Škrinjar, M. G.
2010-04-01
Watson-like integrals for a d-dimensional bcc antiferromagnetic lattice, I_d (\\eta ) =\\frac{1}{\\pi ^d} \\prod _{i = 1}^d \\int _0^{\\pi } \\mathrm{d}x_i \\; \\frac{ \\eta }{\\sqrt{\\eta ^2 - \\prod \
Phase diagram of the triangular-lattice Potts antiferromagnet
Lykke Jacobsen, Jesper; Salas, Jesús; Scullard, Christian R.
2017-08-01
We study the phase diagram of the triangular-lattice Q-state Potts model in the real (Q, v) -plane, where v=e^J-1 is the temperature variable. Our first goal is to provide an obviously missing feature of this diagram: the position of the antiferromagnetic critical curve. This curve turns out to possess a bifurcation point with two branches emerging from it, entailing important consequences for the global phase diagram. We have obtained accurate numerical estimates for the position of this curve by combining the transfer-matrix approach for strip graphs with toroidal boundary conditions and the recent method of critical polynomials. The second goal of this work is to study the corresponding Ap-1 RSOS model on the torus, for integer p=4, 5, \\ldots, 8 . We clarify its relation to the corresponding Potts model, in particular concerning the role of boundary conditions. For certain values of p, we identify several new critical points and regimes for the RSOS model and we initiate the study of the flows between the corresponding field theories.
Masuda, Hiroshi; Okubo, Tsuyoshi; Kawamura, Hikaru
2012-08-03
Motivated by the recent experiment on kagome-lattice antiferromagnets, we study the zero-field ordering behavior of the antiferromagnetic classical Heisenberg model on a uniaxially distorted kagome lattice by Monte Carlo simulations. A first-order transition, which has no counterpart in the corresponding undistorted model, takes place at a very low temperature. The origin of the transition is ascribed to a cooperative proliferation of topological excitations inherent to the model.
Lapinskas, Saulius; Rosengren, Anders
1994-06-01
Using the cluster-variation method we study the phase diagram of the Blume-Emergy-Griffiths (BEG) model on simple cubic and face-centered cubic lattices. For the simple cubic lattice the main attention is paid to reentrant phenomena and ferrimagnetic phases occurring in a certain range of coupling constants. The results are in close agreement with Monte-Carlo data, available for parts of the phase diagram. Several ferrimagnetic phases are obtained in the vicinity of the line in parameter space, at which the model reduces to the antiferromagnetic three-state Potts model. Our results imply the existence of three phase transitions in the antiferromagnetic Potts model on the simple-cubic lattice. The phase diagrams for the BEG model on the face-centered cubic lattice are obtained in the region of antiquadrupolar ordering. Also the several ordered phases of the antiferromagnetic Potts model on this lattice are discussed.
Evidence for a bicritical point in the XXZ Heisenberg antiferromagnet on a simple cubic lattice.
Selke, Walter
2011-04-01
The classical Heisenberg antiferromagnet with uniaxial exchange anisotropy (XXZ model) in a field on a simple cubic lattice is studied with the help of extensive Monte Carlo simulations. We analyze, in particular, various staggered susceptibilities and Binder cumulants and present clear evidence for the triple point of the antiferromagnetic, spin-flop, and paramagnetic phases being a bicritical point with Heisenberg symmetry. Results are compared to previous predictions applying various theoretical approaches.
Evaluation of Watson-like Integrals for Hyper bcc Antiferromagnetic Lattice
Radosevic, S M; Kapor, D V; Pavkov-Hrvojevic, M V; Skrinjar, M G
2010-01-01
Watson-like integrals for a d-dimensional bcc antiferromagnetic lattice I_d(\\eta) and J_d(\\eta) and another two similar integrals are evaluated in an exact way in terms of generalized hypergeometric functions. A simple formula connecting Id and Jd+1 is given along with the differential equations for I_d(\\eta) and J_d(\\eta). An application of I_d and J_d in the theory of the Heisenberg antiferromagnet is discussed, together with possible generalizations to non-integer values of d. Corresponding integrals for sc lattices are also briefly reviewed.
Study of the Antiferromagnetic Blume-Capel Model on kagomé Lattice
Hwang, Chi-Ok; Park, Sojeong; Kwak, Wooseop
2016-09-01
We study the anti-ferromagnetic (AF) Ising model and the AF Blume-Capel (BC) model on the kagomé lattice. Using the Wang-Landau sampling method, we estimate the joint density functions for both models on the lattice, and we obtain the exact critical magnetic fields at zero temperature by using the micro-canonical analysis. We also show the patterns of critical lines for the models from micro-canonical analysis.
Spin superconductivity in the frustrated two-dimensional antiferromagnet in the square lattice
Lima, L. S.
2017-02-01
We use the SU(2) Schwinger boson formalism to study the spin transport in the two-dimensional S = 1 / 2 frustrated Heisenberg antiferromagnet in a square lattice, considering the second-neighbors interactions in the diagonal. We have obtained a spin superfluid behavior for the spin transport to this system similar to obtained recently to the triangular lattice. We consider an antiferromagnetic inter-chain coupling on the diagonal, J2 > 0 , and the nearest-neighbor coupling antiferromagnetic J1 > 0 . We also have in the critical temperature T0, where the correlation length ξ → 0 , that the system suffers a transition from an ordered ground state to a disordered ground state.
Shinaoka, Hiroshi; Tomita, Yusuke; Motome, Yukitoshi
2011-07-22
Motivated by puzzling characteristics of spin-glass transitions widely observed in pyrochlore-based frustrated materials, we investigate the effects of coupling to local lattice distortions in a bond-disordered antiferromagnet on the pyrochlore lattice by extensive Monte Carlo simulations. We show that the spin-glass transition temperature T(f) is largely enhanced by the spin-lattice coupling and, furthermore, becomes almost independent of Δ in a wide range of the disorder strength Δ. The critical property of the spin-glass transition is indistinguishable from that of the canonical Heisenberg spin glass in the entire range of Δ. These peculiar behaviors are ascribed to a modification of the degenerate manifold from a continuous to semidiscrete one by spin-lattice coupling.
McLaughlin, A C; Sher, F; Attfield, J P
2005-08-11
The mechanism of high-transition-temperature (high-T(c)) superconductivity in doped copper oxides is an enduring problem. Antiferromagnetism is established as the competing order, but the relationship between the two states in the intervening 'pseudogap' regime has become a central puzzle. The role of the crystal lattice, which is important in conventional superconductors, also remains unclear. Here we report an anomalous increase of the distance between copper oxide planes on cooling, which results in negative thermal volume expansion, for layered ruthenium copper oxides that have been doped to the boundary of antiferromagnetism and superconductivity. We propose that a crossover between these states is driven by spin ordering in the ruthenium oxide layers, revealing a novel mechanism for negative lattice expansion in solids. The differences in volume and lattice strain between the distinct superconducting and antiferromagnetic states can account for the phase segregation phenomena found extensively in low-doped copper oxides, and show that Cooper pair formation is coupled to the lattice. Unusually large variations of resistivity with magnetic field are found in these ruthenium copper oxides at low temperatures through coupling between the ordered Ru and Cu spins.
The anti-ferromagnetic Ising model on the simplest pure Husimi lattice: An exact solution
Jurčišinová, E., E-mail: jurcisine@saske.sk [Institute of Experimental Physics, SAS, Watsonova 47, 040 01 Košice (Slovakia); Jurčišin, M., E-mail: jurcisin@saske.sk [Institute of Experimental Physics, SAS, Watsonova 47, 040 01 Košice (Slovakia); Bobák, A., E-mail: andrej.bobak@upjs.sk [Department of Theoretical Physics and Astrophysics, Faculty of Science, P.J. Šafárik University, Park Angelinum 9, 040 01 Košice (Slovakia)
2013-11-22
The anti-ferromagnetic spin-1/2 Ising model on the pure Husimi lattice with three sites in the elementary polygon (p=3) and the coordination number z=4 is investigated. It represents the simplest approximation of the anti-ferromagnetic Ising model on the two-dimensional kagome lattice which takes into account effects of frustration. The exact analytical solution of the model is found and discussed. It is proven that the model does not exhibit the first order as well as the second order phase transitions. A detailed analysis of the magnetization properties is performed and the existence of the magnetization plateaus for low temperatures is shown. All possible ground states of the model are found and discussed.
Spin-1/2 Heisenberg Antiferromagnet on the Spatially Anisotropic Kagome Lattice
Schnyder, Andreas; Starykh, Oleg; Balents, Leon
2008-03-01
We study the quasi-one-dimensional limit of the Spin-1/2 quantum antiferromagnet on the Kagome lattice, a model Hamiltonian that might be of relevance for the mineral volborthite [1,2]. The lattice is divided into antiferromagnetic spin-chains (exchange J) that are weakly coupled via intermediate ``dangling'' spins (exchange J'). Using bosonization, renormalization group methods, and current algebra techniques we determine the ground state as a function of J'/J. The case of a strictly one-dimensional Kagome strip is also discussed. [1] Z. Hiroi, M. Hanawa, N. Kobayashi, M. Nohara, Hidenori Takagi, Y. Kato, and M. Takigawa, J. Phys. Soc. Japan 70, 3377 (2001). [2] F. Bert, D. Bono, P. Mendels, F. Ladieu, F. Duc, J.-C. Trumbe, and P. Millet, Phys. Rev. Lett. 95, 087203 (2005).
Solution of the antiferromagnetic Ising model on a tetrahedron recursive lattice.
Jurčišinová, E; Jurčišin, M
2014-03-01
We consider the antiferromagnetic spin-1/2 Ising model on the recursive tetrahedron lattice on which two elementary tetrahedrons are connected at each site. The model represents the simplest approximation of the antiferromagnetic Ising model on the real three-dimensional tetrahedron lattice which takes into account effects of frustration. An exact analytical solution of the model is found and discussed. It is shown that the model exhibits neither the first-order nor the second-order phase transitions. A detailed analysis of the magnetization of the model in the presence of the external magnetic field is performed and the existence of the magnetization plateaus for low temperatures is shown. All possible ground states of the model are found and discussed. The existence of nontrivial singular ground states is proven and exact explicit expressions for them are found.
Monte Carlo Study of the Anisotropic Heisenberg Antiferromagnet on the Triangular Lattice
Stephan, W.; Southern, B. W.
1999-01-01
We report a Monte Carlo study of the classical antiferromagnetic Heisenberg model with easy axis anisotropy on the triangular lattice. Both the free energy cost for long wavelength spin waves as well as for the formation of free vortices are obtained from the spin stiffness and vorticity modulus respectively. Evidence for two distinct Kosterlitz-Thouless types of defect-mediated phase transitions at finite temperatures is presented.
Hida, Kazuo
1995-01-01
The ground state of the square lattice bilayer quantum antiferromagnet with nearest and next-nearest neighbour intralayer interaction is studied by means of the modified spin wave method. For weak interlayer coupling, the ground state is found to be always magnetically ordered while the quantum disordered phase appear for large enough interlayer coupling. The properties of the disordered phase vary according to the strength of the frustration. In the regime of weak frustration, the disordered...
Classical Heisenberg antiferromagnet on a garnet lattice: a Monte Carlo simulation
2000-01-01
We have studied a classical antiferromagnet on a garnet lattice by means of Monte Carlo simulations in an attempt to examine the role of geometrical frustration in Gadolinium Gallium Garnet, Gd3Ga5O12 (GGG). Low-temperature specific heat, magnetisation, susceptibility, the autocorrelation function A(t) and the neutron scattering function S(Q) have been calculated for several models including different types of magnetic interactions and with the presence of an external magnetic field applied a...
Yamagata, Atsushi
1994-01-01
We perform the Monte Carlo simulations of the hard-sphere lattice gas on the simple cubic lattice with nearest neighbour exclusion. The critical activity is estimated, $z_{\\rm c} = 1.0588 \\pm 0.0003$. Using a relation between the hard-sphere lattice gas and the antiferromagnetic Ising model in an external magnetic field, we conclude that there is no re-entrant phase transition of the latter on the simple cubic lattice.
Borovský, Michal; Weigel, Martin; Barash, Lev Yu.; Žukovič, Milan
2016-02-01
The population annealing algorithm is a novel approach to study systems with rough free-energy landscapes, such as spin glasses. It combines the power of simulated annealing, Boltzmann weighted differential reproduction and sequential Monte Carlo process to bring the population of replicas to the equilibrium even in the low-temperature region. Moreover, it provides a very good estimate of the free energy. The fact that population annealing algorithm is performed over a large number of replicas with many spin updates, makes it a good candidate for massive parallelism. We chose the GPU programming using a CUDA implementation to create a highly optimized simulation. It has been previously shown for the frustrated Ising antiferromagnet on the stacked triangular lattice with a ferromagnetic interlayer coupling, that standard Markov Chain Monte Carlo simulations fail to equilibrate at low temperatures due to the effect of kinetic freezing of the ferromagnetically ordered chains. We applied the population annealing to study the case with the isotropic intra- and interlayer antiferromagnetic coupling (J2/|J1| = -1). The reached ground states correspond to non-magnetic degenerate states, where chains are antiferromagnetically ordered, but there is no long-range ordering between them, which is analogical with Wannier phase of the 2D triangular Ising antiferromagnet.
Borovský Michal
2016-01-01
Full Text Available The population annealing algorithm is a novel approach to study systems with rough free-energy landscapes, such as spin glasses. It combines the power of simulated annealing, Boltzmann weighted differential reproduction and sequential Monte Carlo process to bring the population of replicas to the equilibrium even in the low-temperature region. Moreover, it provides a very good estimate of the free energy. The fact that population annealing algorithm is performed over a large number of replicas with many spin updates, makes it a good candidate for massive parallelism. We chose the GPU programming using a CUDA implementation to create a highly optimized simulation. It has been previously shown for the frustrated Ising antiferromagnet on the stacked triangular lattice with a ferromagnetic interlayer coupling, that standard Markov Chain Monte Carlo simulations fail to equilibrate at low temperatures due to the effect of kinetic freezing of the ferromagnetically ordered chains. We applied the population annealing to study the case with the isotropic intra- and interlayer antiferromagnetic coupling (J2/|J1| = −1. The reached ground states correspond to non-magnetic degenerate states, where chains are antiferromagnetically ordered, but there is no long-range ordering between them, which is analogical with Wannier phase of the 2D triangular Ising antiferromagnet.
Quantum phase transition of the randomly diluted heisenberg antiferromagnet on a square lattice
Kato; Todo; Harada; Kawashima; Miyashita; Takayama
2000-05-01
Ground-state magnetic properties of the diluted Heisenberg antiferromagnet on a square lattice are investigated by means of the quantum Monte Carlo method with the continuous-time loop algorithm. It is found that the critical concentration of magnetic sites is independent of the spin size S, and equal to the two-dimensional percolation threshold. However, the existence of quantum fluctuations makes the critical exponents deviate from those of the classical percolation transition. Furthermore, we found that the transition is not universal, i.e., the critical exponents significantly depend on S.
Quantum selection of order in an XXZ antiferromagnet on a Kagome lattice.
Chernyshev, A L; Zhitomirsky, M E
2014-12-05
Selection of the ground state of the kagome-lattice XXZ antiferromagnet by quantum fluctuations is investigated by combining nonlinear spin-wave and real-space perturbation theories. The two methods unanimously favor q=0 over sqrt[3]×sqrt[3] magnetic order in a wide range of the anisotropy parameter 0≤Δ≲0.72. Both approaches are also in accord on the magnitude of the quantum order-by-disorder effect generated by topologically nontrivial, looplike spin-flip processes. A tentative S-Δ phase diagram of the model is proposed.
Two-dimensional-lattice spin models with long-range antiferromagnetic interactions
Romano, S.
1991-10-01
We consider a classical system, consisting of m-component unit vectors (m=2,3), associated with a two-dimensional lattice \\{uk||k∈openZ2\\} and interacting via translationally and rotationally invariant antiferromagnetic pair potentials of the long-range form W=Wjk=ɛ||xj-xk||-puj.uk, p>2, where ɛ is a positive quantity, setting energy and temperature scales (i.e., T*=kBT/ɛ), and xk are the coordinates of the lattice sites. A spin-wave approach predicts orientational disorder (in the thermodynamic limit) at all finite temperatures and for all p>2 this agrees with available rigorous results for p>=4, whereas no such theorems are known in the literature when 22.
Frustrated antiferromagnet on generalized partial line graphs of a honeycomb lattice
Miyahara, Shin; Hotta, Chisa; Kubo, Kenn; Furukawa, Nobuo
2007-03-01
Recently we have proposed generalized partial line graphs on which tight binding models of electronic energy bands realize flat bands [1]. We study Heisenberg antiferromagnets on these structures, which are frustrated and may realize novel ground states. In this report, we focus on a generalized partial line graph created on a honeycomb lattice. The model is a honeycomb lattice composed of A and B-sublattice, where a triangle cluster sits on a site of A-sublattice and a single spin exists on a site of the B-sublattice. We assume the two-types of exchange coupling: J inside the triangle cluster and J' between the cluster and B-sublattice. In the limit J > J' and J J. Phys. Soc. Japan, 74 1918 (2005).
Order and excitations in large-S kagome-lattice antiferromagnets
Chernyshev, A. L.; Zhitomirsky, M. E.
2015-10-01
We systematically investigate the ground-state and the spectral properties of antiferromagnets on a kagomé lattice with several common types of the planar anisotropy: X X Z , single-ion, and out-of-plane Dzyaloshinskii-Moriya. Our main focus is on the role of nonlinear, anharmonic terms, which are responsible for the quantum order-by-disorder effect and for the corresponding selection of the ground-state spin structure in many of these models. The X X Z and the single-ion anisotropy models exhibit a quantum phase transition between the q =0 and the √{3 }×√{3 } states as a function of the anisotropy parameter, offering a rare example of the quantum order-by-disorder fluctuations favoring a ground state which is different from the one selected by thermal fluctuations. The nonlinear terms are also shown to be crucial for a very strong near-resonant decay phenomenon leading to the quasiparticle breakdown in the kagomé-lattice antiferromagnets whose spectra are featuring flat or weakly dispersive modes. The effect is shown to persist even in the limit of large spin values and should be common to other frustrated magnets with flat branches of excitations. Model calculations of the spectrum of the S =5 /2 Fe-jarosite with Dzyaloshinskii-Moriya anisotropy provide a convincing and detailed characterization of the proposed scenario.
Classical Heisenberg antiferromagnet on a garnet lattice: A Monte Carlo simulation
Petrenko, O. A.; Paul, D. McK.
2001-01-01
We have studied a classical antiferromagnet on a garnet lattice by means of Monte Carlo simulations in an attempt to examine the role of geometrical frustration in gadolinium gallium garnet Gd3Ga5O12 (GGG). Low-temperature specific heat, magnetization, susceptibility, the autocorrelation function A(t), and the neutron scattering function S(Q) have been calculated for several models including different types of magnetic interactions and with the presence of an external magnetic field applied along the principal symmetry axes. A model, which includes only nearest-neighbor exchange J1, neither orders down to the lowest temperature nor does it show any tendency towards forming a short-range coplanar spin structure. This model, however, does demonstrate a magnetic field induced ordering below T~0.01J1. In order to reproduce the experimentally observed properties of GGG, the simulated model must include nearest-neighbor exchange interactions and also dipolar forces. The presence of weak next-to-nearest exchange interactions is found to be insignificant. In zero field S(Q) exhibits diffuse magnetic scattering around positions in reciprocal space where antiferromagnetic Bragg peaks appear in an applied magnetic field.
Magnetic excitation spectrum of the square lattice S=1/2 Heisenberg antiferromagnet K2V3O8
Lumsden, M.D.; Nagler, S.E.; Sales, B.C.;
2006-01-01
We have explored the magnetic excitation spectrum of the S=1/2 square lattice Heisenberg antiferromagnet, K2V3O8, using both triple-axis and time-of-flight inelastic neutron scattering. The long-wavelength spin waves are consistent with the previously determined Hamiltonian for this material...
Shuaibu, A. [Department of Physics, Faculty of Science, Universiti Putra Malaysia, 43400 UPM Serdang, Selangor, Malaysia and Physics Department, Faculty of Science, Nigerian Defence Academy, P.M.B 2109, Kaduna (Nigeria); Rahman, M. M. [Physics Department, Faculty of Science, Nigerian Defence Academy, P.M.B 2109, Kaduna (Nigeria)
2014-03-05
We study the low temperature behavior of a triangular lattice quantum spin-1 Heisenberg antiferromagnet with single-site anisotropy by using coordinate Bethe ansatz method. We compute the standard two-particle Hermitian Hamiltonian, and obtain the eigenfunctions and eigenvalue of the system. The obtained results show a number of advantages in comparison with many results.
Hamer, C. J.
2009-06-01
The energy spectra of the two-magnon bound states in the Heisenberg-Ising antiferromagnet on the square lattice are calculated using series expansion methods. The results confirm an earlier spin-wave prediction of Oguchi and Ishikawa that the bound states vanish into the continuum before the isotropic Heisenberg limit is reached.
Spin-Ice State of the Quantum Heisenberg Antiferromagnet on the Pyrochlore Lattice
Huang, Yuan; Chen, Kun; Deng, Youjin; Prokof'ev, Nikolay; Svistunov, Boris
2016-04-01
We study the low-temperature physics of the SU(2)-symmetric spin-1 /2 Heisenberg antiferromagnet on a pyrochlore lattice and find "fingerprint" evidence for the thermal spin-ice state in this frustrated quantum magnet. Our conclusions are based on the results of bold diagrammatic Monte Carlo simulations, with good convergence of the skeleton series down to the temperature T /J =1 /6 . The identification of the spin-ice state is done through a remarkably accurate microscopic correspondence for the static structure factor between the quantum Heisenberg, classical Heisenberg, and Ising models at all accessible temperatures, and the characteristic bowtie pattern with pinch points observed at T /J =1 /6 . The dynamic structure factor at real frequencies (obtained by the analytic continuation of numerical data) is consistent with diffusive spinon dynamics at the pinch points.
Spin-Ice State of the Quantum Heisenberg Antiferromagnet on the Pyrochlore Lattice.
Huang, Yuan; Chen, Kun; Deng, Youjin; Prokof'ev, Nikolay; Svistunov, Boris
2016-04-29
We study the low-temperature physics of the SU(2)-symmetric spin-1/2 Heisenberg antiferromagnet on a pyrochlore lattice and find "fingerprint" evidence for the thermal spin-ice state in this frustrated quantum magnet. Our conclusions are based on the results of bold diagrammatic Monte Carlo simulations, with good convergence of the skeleton series down to the temperature T/J=1/6. The identification of the spin-ice state is done through a remarkably accurate microscopic correspondence for the static structure factor between the quantum Heisenberg, classical Heisenberg, and Ising models at all accessible temperatures, and the characteristic bowtie pattern with pinch points observed at T/J=1/6. The dynamic structure factor at real frequencies (obtained by the analytic continuation of numerical data) is consistent with diffusive spinon dynamics at the pinch points.
Bond operator theory for the frustrated anisotropic Heisenberg antiferromagnet on a square lattice
Pires, A.S.T., E-mail: antpires@fisica.ufmg.br [Departamento de Fisica, Universidade Federal de Minas Gerais, Belo Horizonte, Cp 702, 30123-970 MG (Brazil)
2012-07-15
The quantum anisotropic antiferromagnetic Heisenberg model with single ion anisotropy, spin S=1 and up to the next-next-nearest neighbor coupling (the J{sub 1}-J{sub 2}-J{sub 3} model) on a square lattice, is studied using the bond-operator formalism in a mean field approximation. The quantum phase transitions at zero temperature are obtained. The model features a complex T=0 phase diagram, whose ordering vector is subject to quantum corrections with respect to the classical limit. The phase diagram shows a quantum paramagnetic phase situated among Neel, spiral and collinear states. - Highlights: Black-Right-Pointing-Pointer The quantum phase transition at zero temperature is studied. Black-Right-Pointing-Pointer The phase diagram up to the next-next-nearest neighbor coupling is calculated. Black-Right-Pointing-Pointer The energy gap is calculated in several regions of the phase diagram.
NMR study of pyrochlore lattice antiferromagnet, melanothallite Cu2OCl2
Nishiyama, Masahide; Oyamada, Akira; Itou, Tetsuaki; Maegawa, Satoru; Okabe, Hirotaka; Akimitsu, Jun
2011-09-01
The melanothallite Cu2OCl2 is a new example of pyrochlore-like antiferromagnet, which is composed of 3d transition metal electrons. We performed Cu- and Cl-NMR experiments on powder samples of Cu2OCl2 below transition temperature TN = 70 K and we observed six resonant peaks of Cu nuclei, which are composed of three symmetric peaks corresponding to 63Cu and three corresponding to 65Cu. The Cu nuclei feel the strong hyperfine fields because of ordered magnetic moments and the electric field gradients. We determined the spin structure by analyzing the Cu-NMR spectra. The melanothallite has an all-in-all-out spin structure. The spin lattice relaxation rates T1-1 of Cu- and Cl-NMR in the ordered phase are proportional to the temperature; This suggests that although long-range ordering occurs at rather high temperature, the large spin fluctuations caused by the geometrical frustration still remain.
Experience with low-alpha lattices at the Diamond Light Source
Martin, I. P. S.; Rehm, G.; Thomas, C.; Bartolini, R.
2011-04-01
In this paper we present the experience at Diamond Light Source in the design, implementation, and operation of low momentum compaction factor lattices for the generation of short x-ray pulses and coherent THz radiation. The effects of higher-order terms in the expansion of the momentum compaction factor on beam dynamics are reviewed from a theoretical point of view, and the details of both high- and low-emittance solutions at Diamond are discussed. Measurements taken to characterize the lattices under a variety of machine conditions are presented, along with the practical limitations that exist as the momentum compaction factor is made to approach zero.
Opal-like photonic crystal with diamond lattice
Garcia Santamaria, F; López, C; Meseguer, F; Miyazaki, H T; Sánchez-Dehesa, J
2002-01-01
In this contribution, a method to fabricate a diamond structure with a complete PBG in the near infrared is proposed. The procedure starts by building an opal composed of two types of microspheres (organic and inorganic) in a body-centered-cubic symmetry by means of a micro- robotic technique. Then, the organic particles may be selectively removed to obtain a diamond structure of inorganic particles. Once this structure is assembled its filling fraction may be controlled by sintering. Subsequently this template can be infiltrated with an adequate high refractive index material. In this way, the method can be extended to make diamond inverse opals of, for instance, silicon with gap to mid gap ratios as large as 13% for moderate filling fractions. An overview of micromanipulation as well as previous experimental results will be offered to show the feasibility of this method. (24 refs).
Melting of Three-Sublattice Order in Easy-Axis Antiferromagnets on Triangular and Kagome Lattices.
Damle, Kedar
2015-09-18
When the constituent spins have an energetic preference to lie along an easy axis, triangular and kagome lattice antiferromagnets often develop long-range order that distinguishes the three sublattices of the underlying triangular Bravais lattice. In zero magnetic field, this three-sublattice order melts either in a two-step manner, i.e., via an intermediate phase with power-law three-sublattice order controlled by a temperature-dependent exponent η(T)∈(1/9,1/4), or via a transition in the three-state Potts universality class. Here, I predict that the uniform susceptibility to a small easy-axis field B diverges as χ(B)∼|B|^{-[(4-18η)/(4-9η)]} in a large part of the intermediate power-law ordered phase [corresponding to η(T)∈(1/9,2/9)], providing an easy-to-measure thermodynamic signature of two-step melting. I also show that these two melting scenarios can be generically connected via an intervening multicritical point and obtain numerical estimates of multicritical exponents.
Optical Signatures of Antiferromagnetic Ordering of Fermionic Atoms in an Optical Lattice
Francisco Cordobes Aguilar
2014-09-01
Full Text Available We show how off-resonant light scattering can provide quantitative information on antiferromagnetic ordering of a two-species fermionic atomic gas in a tightly-confined two-dimensional optical lattice. We analyze the emerging magnetic ordering of atoms in the mean-field and in random phase approximations and show how the many-body static and dynamic correlations, evaluated in the standard Feynman-Dyson perturbation series, can be detected in the scattered light signal. The staggered magnetization reveals itself in the magnetic Bragg peaks of the individual spin components. These magnetic peaks, however, can be considerably suppressed in the absence of a true long-range antiferromagnetic order. The light scattered outside the diffraction orders can be collected by a lens with highly improved signal-to-shot-noise ratio when the diffraction maxima are blocked. The collective and single-particle excitations are identified in the spectrum of the scattered light. We find that the spin-conserving and spin-exchanging atomic transitions convey information on density, longitudinal spin, and transverse spin correlations. The different correlations and scattering processes exhibit characteristic angular distribution profiles for the scattered light, and e.g., the diagnostic signal of transverse spin correlations could be separated from the optical response by the scattering direction, frequency, or polarization. We also analyze the detection accuracy by estimating the number of required measurements, constrained by the heating rate that is determined by inelastic light-scattering events. The imaging technique could be extended to the two-species fermionic states in other regions of the phase diagram where the ground-state properties are still not fully understood.
Monte carlo simulation study of the square lattice S=1/2 quantum heisenberg antiferromagnet
Kim, J K
1999-01-01
For the two dimensional S= 1/2 isotopic quantum Heisenberg antiferromagnet on a square lattice, we report our results of an extensive quantum Monte Carlo simulation for various physical observables such as the correlation length xi, the staggered magnetic susceptibility chi sub S sub T , the structure factor peak value S(Q), the internal energy epsilon, and the uniform susceptibility chi sub u. We find that chi sub S sub T approx chi sup 2 T and S(Q) approx xi sup 2 T sup 2 , in agreement with the predictions of the conventional theory but in disagreement with recent experiments. Our estimate of the spin stiffness constant rho sub s and spin wave velocity c, from the low temperature behavior of the chi sub u is shown to be consistent with the theoretical prediction of the low temperature behavior of the epsilon, and of the xi provided an additional correction up to T sup 2. However, our data are definitely inconsistent with the scenario of the crossover for the xi.
Search for the Heisenberg spin glass on rewired cubic lattices with antiferromagnetic interaction
Surungan, Tasrief
2016-10-01
Spin glass (SG) is a typical magnetic system which is mainly characterized by a frozen random spin orientation at low temperatures. Frustration and randomness are considered to be the key ingredients for the existence of SGs. Previously, Bartolozzi et al. [Phys. Rev. B73, 224419 (2006)] found that the antiferromagnetic (AF) Ising spins on scale free network (SFN) exhibited SG behavior. This is purely AF system, a new type of SG different from the canonical one which requires the presence of both FM and AF couplings. In this new system, frustration is purely due to a topological factor and its randomness is brought by irregular connectivity. Recently, it was reported that the AF Heisenberg model on SFN exhibited SG behavior [Surungan et al., JPCS, 640, 012005 (2015)/doi:10.1088/1742-6596/640/1/012005]. In order to accommodate the notion of spatial dimension, we further investigated this type of system by studying an AF Heisenberg model on rewired cubic lattices, constructed by adding one extra bond randomly connecting each spin to one of its next-nearest neighbors. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter to search for the existence of SG phase.
Search for the Heisenberg spin glass on rewired square lattices with antiferromagnetic interaction
Surungan, Tasrief; Bansawang B., J.; Tahir, Dahlang
2016-03-01
Spin glass (SG) is a typical magnetic system with frozen random spin orientation at low temperatures. The system exhibits rich physical properties, such as infinite number of ground states, memory effect, and aging phenomena. There are two main ingredients considered to be pivotal for the existence of SG behavior, namely, frustration and randomness. For the canonical SG system, frustration is led by the presence of competing interaction between ferromagnetic (FM) and antiferromagnetic (AF) couplings. Previously, Bartolozzi et al. [Phys. Rev. B73, 224419 (2006)], reported the SG properties of the AF Ising spins on scale free network (SFN). It is a new type of SG, different from the canonical one which requires the presence of both FM and AF couplings. In this new system, frustration is purely caused by the topological factor and its randomness is related to the irregular connectvity. Recently, Surungan et. al. [Journal of Physics: Conference Series, 640, 012001 (2015)] reported SG bahavior of AF Heisenberg model on SFN. We further investigate this type of system by studying an AF Heisenberg model on rewired square lattices. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter to search for the existence of SG phase.
Lattice and spin dynamics in a low-symmetry antiferromagnet NiWO4
Prosnikov, M. A.; Davydov, V. Yu.; Smirnov, A. N.; Volkov, M. P.; Pisarev, R. V.; Becker, P.; Bohatý, L.
2017-07-01
Lattice and magnetic dynamics of NiWO4 single crystals were studied with the use of polarized Raman spectroscopy in a wide temperature range of 10-300 K including the antiferromagnetic ordering temperature TN=62 K. Static magnetic measurements were used for characterizing the single crystals. All Raman-active phonons predicted by the group theory were observed and characterized. Magnetic symmetry analysis was used to determine possible magnetic space groups for NiWO4 which can be also applied to any other isostructural crystal with the same magnetic propagation vector k =(1 /2 ,0 ,0 ) . Although the magnetic structure of NiWO4 is relatively simple, a rich set of narrow and broad magnetic excitations with different polarization properties and temperature behavior in the very broad frequency range of 10-200 cm-1 was observed, with some modes surviving at temperatures much higher than TN up to 220 K. Part of the magnetic excitations were identified as acoustic and optical spin-wave branches which allowed us to construct exchange structure and estimate exchange and anisotropy constants with the use of linear spin-wave theory.
Spin dynamics of S = 1/2 kagome lattice antiferromagnets observed by high-field ESR
Ohta, Hitoshi [Molecular Photoscience Research Center, Kobe University, Kobe 657-8501 (Japan); Graduate School of Science, Kobe University, Kobe 657-8501 (Japan); Zhang, Wei-min [Graduate School of Science, Kobe University, Kobe 657-8501 (Japan); Okubo, Susumu; Fujisawa, Masashi [Molecular Photoscience Research Center, Kobe University, Kobe 657-8501 (Japan); Sakurai, Takahiro [Center for Supports to Research and Education Activities, Kobe University, Kobe 657-8501 (Japan); Okamoto, Yoshihiko; Yoshida, Hiroyuki; Hiroi, Zenji [Institute for Solid State Physics (ISSP), University of Tokyo, Kashiwa, Chiba 277-8581 (Japan)
2010-03-15
Due to the existence of strong spin frustration in a system, the spin dynamics of S = 1/2 kagome lattice antiferromagnet at low temperature has attracted much interest. High-field ESR has been measured on its model substances, Cu{sub 3}V{sub 2}O{sub 7}(OH){sub 2} . 2H{sub 2}O (volborthite) and BaCu{sub 3}V{sub 2}O{sub 3}(OH){sub 2} (vesignieite), down to 1.8 K using pulsed magnetic fields up to 16 T. The measurements are performed for 160 and 315 GHz using polycrys-talline samples. Although both samples showed the g-shift and the change of linewidth at low temperature, volborthite showed a small gap excitation of the order of 40 GHz (1.9 K) while vesignieite showed a paramagnetic behavior down to 1.9 K. Observed difference will be discussed in connection with the crystal structure, and the possible spin liquid state in vesignieite will be discussed. (Abstract Copyright [2010], Wiley Periodicals, Inc.)
Spin-1/2 Heisenberg J1-J2 antiferromagnet on the kagome lattice
Iqbal, Yasir; Poilblanc, Didier; Becca, Federico
2015-01-01
We report variational Monte Carlo calculations for the spin-1/2 Heisenberg model on the kagome lattice in the presence of both nearest-neighbor J1 and next-nearest-neighbor J2 antiferromagnetic superexchange couplings. Our approach is based upon Gutzwiller projected fermionic states that represent a flexible tool to describe quantum spin liquids with different properties (e.g., gapless and gapped). We show that, on finite clusters, a gapped Z2 spin liquid can be stabilized in the presence of a finite J2 superexchange, with a substantial energy gain with respect to the gapless U (1 ) Dirac spin liquid. However, this energy gain vanishes in the thermodynamic limit, implying that, at least within this approach, the U (1 ) Dirac spin liquid remains stable in a relatively large region of the phase diagram. For J2/J1≳0.3 , we find that a magnetically ordered state with q =0 overcomes the magnetically disordered wave functions, suggesting the end of the putative gapless spin-liquid phase.
GdPtPb: A noncollinear antiferromagnet with distorted kagome lattice
Manni, S.; Bud'ko, Sergey L.; Canfield, Paul C.
2017-08-01
In the spirit of searching for Gd-based, frustrated, rare earth magnets, we have found antiferomagnetism (AF) in GdPtPb, which crystallizes in the ZrNiAl-type structure that has a distorted kagome lattice of Gd triangles. Single crystals were grown and investigated using structural, magnetic, transport, and thermodynamic measurements. GdPtPb orders antiferromagnetically at 15.5 K, arguably with a planar, noncollinear structure. The high temperature magnetic susceptibility data reveal an "anti-frustration" behavior having a frustration parameter, |f | =|Θ | /TN=0.25 , which can be explained by mean field theory within a two-sublattice model. Study of the magnetic phase diagram down to T =1.8 K reveals a change of magnetic structure through a metamagnetic transition at around 20 kOe and the disappearance of the AF ordering near 140 kOe. In total, our work indicates that GdPtPb can serve as an example of a planar, noncollinear AF with a distorted kagome magnetic sublattice.
Current loops and fluctuations in the zero-range process on a diamond lattice
Villavicencio-Sanchez, R.; Harris, R. J.; Touchette, H.
2012-07-01
We study the zero-range process on a simple diamond lattice with open boundary conditions and determine the conditions for the existence of loops in the mean current. We also perform a large deviation analysis for fluctuations of partial and total currents and check the validity of the Gallavotti-Cohen fluctuation relation for these quantities. In this context, we show that the fluctuation relation is not satisfied for partial currents between sites even if it is satisfied for the total current flowing between the boundaries. Finally, we extend our methods to study a chain of coupled diamonds and demonstrate co-existence of mean current regimes.
Control of the third dimension in copper-based square-lattice antiferromagnets
Goddard, Paul A.; Singleton, John; Franke, Isabel; Möller, Johannes S.; Lancaster, Tom; Steele, Andrew J.; Topping, Craig V.; Blundell, Stephen J.; Pratt, Francis L.; Baines, C.; Bendix, Jesper; McDonald, Ross D.; Brambleby, Jamie; Lees, Martin R.; Lapidus, Saul H.; Stephens, Peter W.; Twamley, Brendan W.; Conner, Marianne M.; Funk, Kylee; Corbey, Jordan F.; Tran, Hope E.; Schlueter, J. A.; Manson, Jamie L.
2016-03-01
Using a mixed-ligand synthetic scheme, we create a family of quasi-two-dimensional antiferromagnets, namely, [Cu(HF2)(pyz)(2)]ClO4 [pyz = pyrazine], [CuL2(pyz)(2)](ClO4)(2) [L = pyO = pyridine-N-oxide and 4-phpy-O = 4-phenylpyridine-N-oxide. These materials are shown to possess equivalent two-dimensional [Cu(pyz)(2)](2+) nearly square layers, but exhibit interlayer spacings that vary from 6.5713 to 16.777 angstrom, as dictated by the axial ligands. We present the structural and magnetic properties of this family as determined via x-ray diffraction, electron-spin resonance, pulsed-and quasistatic-field magnetometry and muon-spin rotation, and compare them to those of the prototypical two-dimensional magnetic polymer Cu(pyz)(2)(ClO4)(2). We find that, within the limits of the experimental error, the two-dimensional, intralayer exchange coupling in our family of materials remains largely unaffected by the axial ligand substitution, while the observed magnetic ordering temperature (1.91 K for the material with the HF2 axial ligand, 1.70 K for the pyO and 1.63 K for the 4-phpy-O) decreases slowly with increasing layer separation. Despite the structural motifs common to this family and Cu(pyz)(2)(ClO4)(2), the latter has significantly stronger two-dimensional exchange interactions and hence a higher ordering temperature. We discuss these results, as well as the mechanisms that might drive the long-range order in these materials, in terms of departures from the ideal S = 1/2 two-dimensional square-lattice Heisenberg antiferromagnet. In particular, we find that both spin-exchange anisotropy in the intralayer interaction and interlayer couplings (exchange, dipolar, or both) are needed to account for the observed ordering temperatures, with the intralayer anisotropy becoming more important as the layers are pulled further apart.
Yamane, Haruki; Kobayashi, Masanobu
2014-01-01
The influence of two-dimensional array structures (hexagonal anti-dot lattices) on magneto-optical (MO) properties was investigated in perpendicular antiferromagnetically coupled Co80Pt20 stacked films containing ZnO optical interference layers. Antiferromagnetic exchange coupling was generated in a [CoPt/Ru/CoPt] tri-layered structure, and anti-dot lattices were formed on both CoPt layers. The exchange coupling between the CoPt layers across a very thin 0.46-nm Ru interlayer was maintained even after nanofabrication. Characteristic MO hysteresis loops were measured by a 405-nm wavelength incident light on samples containing a 50-nm ZnO optical interference layer. The anti-dot lattice with a 200-nm diameter hole exhibited an increase in the residual Kerr rotation angle owing to the antiparallel magnetization alignment of the CoPt layers. Furthermore, compared with samples without the interference layer, the figure of merit for the anti-dot lattice with a 200-nm diameter hole was enhanced by inserting a 100-nm ZnO interference layer. These improvements are attributed to MO interference effects inside the stacked films.
Lima, L. S.
2017-04-01
We use the SU(N) Schwinger boson formalism to study the spin transport in the S=1 biquadratic frustrated Heisenberg antiferromagnetic model in the triangular lattice, considering the next-nearest-neighbors interactions J2. We have obtained a jump in the spin conductivity in the point of cusp of the phase diagram - η vs. - α of the model at T=0, which represents the force of the biquadratic coupling versus the next-nearest-neighbor coupling (K vs. J2). We have obtained also a superfluid behavior for the spin transport in the DC limit for this system similar to ones recently obtained for other two-dimensional frustrated spin systems. We consider all the couplings, first and second couplings as antiferromagnetic.
Inaba, Kensuke; Yamashita, Makoto
2010-10-22
We propose a simple method to detect the antiferromagnetic (AF) state of fermionic atoms in an optical lattice by combining a time-of-flight (TOF) imaging method and a Feshbach resonance. In this scheme, the nontrivial dynamics of fermionic atoms during the imaging process works as a probe with respect to the breaking of the translational symmetry in the AF state. Precise numerical simulations demonstrate that the characteristic oscillatory dynamics induced by the scattering process that transfers an AF ordering vector appears in TOF images, which can be easily observed experimentally.
Magnetic properties of the S =1/2 honeycomb lattice antiferromagnet 2 -Cl -3 ,6 -F2-V
Okabe, Toshiki; Yamaguchi, Hironori; Kittaka, Shunichiro; Sakakibara, Toshiro; Ono, Toshio; Hosokoshi, Yuko
2017-02-01
We successfully synthesized single crystals of the verdazyl radical 2 -Cl -3 ,6 -F2-V [=3-(2-chloro-3,6-difluorophenyl)-1,5-diphenylverdazyl], which is a rare model compound with an S =1/2 Heisenberg antiferromagnetic (HAF) honeycomb lattice. Ab initio molecular orbital calculations indicate two dominant AF interactions, forming a slightly distorted honeycomb lattice. We explain the magnetic susceptibility and the magnetization curve up to the saturation field based on the expected spin model using the quantum Monte Carlo method. In the low-temperature regions, we found a phase transition to an AF ordered state at about 0.77 K for the zero field and obtained the magnetic field-temperature phase diagram from the magnetic susceptibility and the specific heat for various magnetic fields. Through the analysis considering the effect of lattice distortion on magnetic behavior, we confirm that the lattice distortion of the present model is small enough that it does not affect the intrinsic behavior of the uniform S =1/2 HAF honeycomb lattice.
Spin frustration and magnetic ordering in triangular lattice antiferromagnet Ca3CoNb2O9
Dai, Jia; Zhou, Ping; Wang, Peng-Shuai; Pang, Fei; Munsie, Tim J.; Luke, Graeme M.; Zhang, Jin-Shan; Yu, Wei-Qiang
2015-12-01
We synthesized a quasi-two-dimensional distorted triangular lattice antiferromagnet Ca3CoNb2O9, in which the effective spin of Co2+ is 1/2 at low temperatures, whose magnetic properties were studied by dc susceptibility and magnetization techniques. The x-ray diffraction confirms the quality of our powder samples. The large Weiss constant θCW˜ -55 K and the low Neel temperature TN˜ 1.45 K give a frustration factor f = | θCW/TN | ≈ 38, suggesting that Ca3CoNb2O9 resides in strong frustration regime. Slightly below TN, deviation between the susceptibility data under zero-field cooling (ZFC) and field cooling (FC) is observed. A new magnetic state with 1/3 of the saturate magnetization Ms is suggested in the magnetization curve at 0.46 K. Our study indicates that Ca3CoNb2O9 is an interesting material to investigate magnetism in triangular lattice antiferromagnets with weak anisotropy. Project supported by the National Natural Science Foundation of China (Grant Nos. 11374364 and 11222433), the National Basic Research Program of China (Grant No. 2011CBA00112). Research at McMaster University supported by the Natural Sciences and Engineering Research Council. Work at North China Electric Power University supported by the Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry.
Mechanical behavior of regular open-cell porous biomaterials made of diamond lattice unit cells.
Ahmadi, S M; Campoli, G; Amin Yavari, S; Sajadi, B; Wauthle, R; Schrooten, J; Weinans, H; Zadpoor, A A
2014-06-01
Cellular structures with highly controlled micro-architectures are promising materials for orthopedic applications that require bone-substituting biomaterials or implants. The availability of additive manufacturing techniques has enabled manufacturing of biomaterials made of one or multiple types of unit cells. The diamond lattice unit cell is one of the relatively new types of unit cells that are used in manufacturing of regular porous biomaterials. As opposed to many other types of unit cells, there is currently no analytical solution that could be used for prediction of the mechanical properties of cellular structures made of the diamond lattice unit cells. In this paper, we present new analytical solutions and closed-form relationships for predicting the elastic modulus, Poisson׳s ratio, critical buckling load, and yield (plateau) stress of cellular structures made of the diamond lattice unit cell. The mechanical properties predicted using the analytical solutions are compared with those obtained using finite element models. A number of solid and porous titanium (Ti6Al4V) specimens were manufactured using selective laser melting. A series of experiments were then performed to determine the mechanical properties of the matrix material and cellular structures. The experimentally measured mechanical properties were compared with those obtained using analytical solutions and finite element (FE) models. It has been shown that, for small apparent density values, the mechanical properties obtained using analytical and numerical solutions are in agreement with each other and with experimental observations. The properties estimated using an analytical solution based on the Euler-Bernoulli theory markedly deviated from experimental results for large apparent density values. The mechanical properties estimated using FE models and another analytical solution based on the Timoshenko beam theory better matched the experimental observations. Copyright © 2014 Elsevier Ltd
Critical behavior of Gaussian model on diamond-type hierarchical lattices
孔祥木; 李崧
1999-01-01
It is proposed that the Gaussian type distribution constant bqi in the Gaussian model depends on the coordination number qi of site i, and that the relation bqi/bqj = qi/qj holds among bqi’s. The Gaussian model is then studied on a family of the diamond-type hierarchical （or DH） lattices, by the decimation real-space renormalization group following spin-resealing method. It is found that the magnetic property of the Gaussian model belongs to the same universal class, and that the critical point K* and the critical exponent v are given by K*= bqi/qi and v=1/2, respectively.
Okubo, Tsuyoshi; Chung, Sungki; Kawamura, Hikaru
2012-01-06
Ordering of the frustrated classical Heisenberg model on the triangular lattice with an incommensurate spiral structure is studied under magnetic fields by means of a mean-field analysis and a Monte Carlo simulation. Several types of multiple-q states including the Skyrmion-lattice state is observed in addition to the standard single-q state. In contrast to the Dzyaloshinskii-Moriya interaction driven system, the present model allows both Skyrmions and anti-Skyrmions, together with a new thermodynamic phase where Skyrmion and anti-Skyrmion lattices form a domain state.
Critical slowing down of the Gaussian spin system on diamond-type hierarchical lattices
朱建阳; 朱涵
2003-01-01
Based on the single-spin transition critical dynamics, we have investigated the critical slowing down of the Gaussian spin model situated on the fractal family of diamond-type hierarchical lattices. We calculate the dynamical critical exponent z and the correlation-length critical exponent v using the dynamical decimation renormalization-group technique. The result, together with some earlier ones, suggests us to conclude that on a wide range of geometries, zv = 1is the general relationship, while the two exponents depend on the specific structure. However, we have investigated for various lattices in an earlier paper, the system studied in this paper shows highly universal z = 1/v = 2 independent of the structure and the dimensionality.
Antiferromagnetic and Orbital Ordering on a Diamond Lattice Near Quantum Criticality
Plumb, K. W.; Morey, J. R.; Rodriguez-Rivera, J. A.; Wu, Hui; Podlesnyak, A. A.; McQueen, T. M.; Broholm, C. L.
2016-10-01
We present neutron scattering measurements on powder samples of the spinel FeSc2S4 that reveal a previously unobserved magnetic ordering transition occurring at 11.8(2) K. Magnetic ordering occurs subsequent to a subtle cubic-to-tetragonal structural transition that distorts Fe coordinating sulfur tetrahedra and lifts the orbital degeneracy. The orbital ordering is not truly long ranged, but occurs over finite-sized domains that limit magnetic correlation lengths. The application of 1 GPa hydrostatic pressure appears to destabilize this Néel state, reducing the transition temperature to 8.6(8) K and redistributing magnetic spectral weight to higher energies. The relative magnitudes of ordered ⟨m ⟩2=3.1 (2 ) μB2 and fluctuating moments ⟨δ m ⟩=13 (1 ) μB2 show that the magnetically ordered state of FeSc2 S4 is drastically renormalized and close to criticality.
Study on ceramic photonic bandgap structure with three-dimensional diamond lattice
Haiqing Yin; Wenbin Cao; Y. Miyamoto
2006-01-01
A novel process, which was based on powder injection molding, was investigated for the fabrication of ceramic photonic bandgap structure with three-dimensional diamond lattice. The SiO2-TiO2 ceramic powder was mixed with a water-soluble agent to produce slurry. The slurry was then injected into an epoxy mold with inverse diamond lattice, fabricated by the stereolitographic rapid prototyping process. To increase the density of the green compact, cold isostatic pressing was applied on the unit. Using thermal debinding, the water-soluble agent and the epoxy were extracted at 360 and 650 K, respectively. Sintering was immediately done at 950 K for 5 h and the desired three-dimensional ceramic structure was obtained. The calculated band diagram for this structure indicated the existence of an absolute photonic bandgap for all wave vectors. At 14.7-18.5 GHz, a complete band gap was located with a maximum attenuation of 30 dB at 17 GHz, when transmission was measured in the 〈100〉 direction between 10 and 20 GHz.
N Rahimipour
2015-07-01
Full Text Available The classical J1-J2 Heisenberg model on bipartite lattice exhibits "Neel" order. However if the AF interactions between the next nearest neighbor(nnn are increased with respect to the nearest neighbor(nn, the frustration effect arises. In such situations, new phases such as ordered phases with coplanar or spiral ordering and disordered phases such as spin liquids can arise. In this paper we use the self-consistent Gaussian approximation to study the J1-J2 Heisenberg model in honeycomb and diamond lattices. We find the spin liquid phases such as ring-liquid and pancake-liquid in honeycomb lattice.Also for diamond lattice we show that the degeneracy of ground state can be lifted by thermal fluctuations through the order by disorder mechanism.
Oh, Joosung; Le, Manh Duc; Jeong, Jaehong; Lee, Jung-hyun; Woo, Hyungje; Song, Wan-Young; Perring, T. G.; Buyers, W. J. L.; Cheong, S.-W.; Park, Je-Geun
2013-12-01
The breakdown of magnons, the quasiparticles of magnetic systems, has rarely been seen. By using an inelastic neutron scattering technique, we report the observation of spontaneous magnon decay in multiferroic LuMnO3, a simple two dimensional Heisenberg triangular lattice antiferromagnet, with large spin S=2. The origin of this rare phenomenon lies in the nonvanishing cubic interaction between magnons in the spin Hamiltonian arising from the noncollinear 120° spin structure. We observed all three key features of the nonlinear effects as theoretically predicted: a rotonlike minimum, a flat mode, and a linewidth broadening, in our inelastic neutron scattering measurements of single crystal LuMnO3. Our results show that quasiparticles in a system hitherto thought of as “classical” can indeed break down.
Shimokawa, Tokuro; Kawamura, Hikaru
2016-11-01
Thermal properties of the S = 1/2 kagome Heisenberg antiferromagnet at low temperatures are investigated by means of the Hams-de Raedt method for clusters of up to 36 sites possessing a full symmetry of the lattice. The specific heat exhibits, in addition to the double peaks, the third and the fourth peaks at lower temperatures. With decreasing the temperature, the type of the magnetic short-range order (SRO) changes around the third-peak temperature from the √{3} × √{3} to the q = 0 states, suggesting that the third peak of the specific heat is associated with a crossover phenomenon between the spin-liquid states with distinct magnetic SRO. Experimental implications are discussed.
Jurčišinová, E.; Jurčišin, M.
2016-09-01
The antiferromagnetic spin-1 Ising model is studied on the Husimi lattice constructed from elementary triangles with coordination number z = 4. It is found that the model has a unique solution for arbitrary values of the magnetic field as well as for all temperatures. A detailed analysis of the magnetization is performed and it is shown that in addition to the standard plateau-like ground states, the model also contains well-defined single-point ground states related to definite values of the magnetic field. Exact values of the residual entropies for all ground states are found. The properties of the susceptibility and the specific heat of the model are also discussed. The existence of the Schottky-type behavior of the specific heat and the strong magnetocaloric effect for low enough temperatures and for the external magnetic field close to the values at which the single-point ground states exist are identified.
Oh, Joosung; Le, Manh Duc; Jeong, Jaehong; Lee, Jung-hyun; Woo, Hyungje; Song, Wan-Young; Perring, T G; Buyers, W J L; Cheong, S-W; Park, Je-Geun
2013-12-20
The breakdown of magnons, the quasiparticles of magnetic systems, has rarely been seen. By using an inelastic neutron scattering technique, we report the observation of spontaneous magnon decay in multiferroic LuMnO3, a simple two dimensional Heisenberg triangular lattice antiferromagnet, with large spin S=2. The origin of this rare phenomenon lies in the nonvanishing cubic interaction between magnons in the spin Hamiltonian arising from the noncollinear 120° spin structure. We observed all three key features of the nonlinear effects as theoretically predicted: a rotonlike minimum, a flat mode, and a linewidth broadening, in our inelastic neutron scattering measurements of single crystal LuMnO3. Our results show that quasiparticles in a system hitherto thought of as "classical" can indeed break down.
Hirose, Yuhei; Miura, Shoma; Yasuda, Chitoshi; Fukumoto, Yoshiyuki
2017-08-01
Quantum Monte Carlo (QMC) simulations are performed to study ground-state properties of a mixed spin-1 and spin-1/2 Lieb-lattice Heisenberg antiferromagnet, in order to get further insight beyond the modified spin-wave (MSW) study reported in [https://doi.org/10.7566/JPSJ.86.014002" xlink:type="simple">J. Phys. Soc. Jpn. 86, 014002 (2017)]. It is confirmed that the MSW results are in good agreement with the QMC results. In particular, the scaling relation found in the MSW study, which argues that sublattice spin reductions are inversely proportional to the sublattice sizes, is observed in our QMC simulation. We present a rigorous proof for spontaneous sublattice magnetizations induced by an infinitesimal uniform magnetic field. The calculation process in the MSW theory is reexamined to clarify the mathematical structure behind the scaling relation for sublattice long-range orders.
A. B. Babaev
2015-01-01
Full Text Available Using Monte-Carlo simulations, we investigated phase transitions and frustrations in the three-state Potts model on a triangular lattice with allowance for antiferromagnetic exchange interactions between nearest- neighbors J1 and next- nearest- neighbors J2. The ratio of the next-nearest- neighbor and nearest- neighbor exchange constants r=J2/J1 is chosen within the 0÷2 range. Based on the analysis of the entropy, specific heat, system state density function, and fourth order Binder cumulants, the phase transitions in the Potts model with interactions J1<0 and J2<0 are shown to be found in value ranges of 0 r<0.2 and 1.0
Murtazaev, Akai K.; Babaev, Albert B.; Magomedov, Magomed A.; Kassan-Ogly, Felix A.; Proshkin, Alexey I.
2016-11-01
Using Monte Carlo simulations, we investigated phase transitions and frustrations in the three-state Potts model on a triangular lattice with allowance for antiferromagnetic exchange interactions between nearest-neighbors J1 and next-nearest-neighbors J2. The ratio of the next-nearest-neighbor and nearest-neighbor exchange constants r=J2/J1 is chosen within the range of 0≤r≤2. Based on the analysis of the entropy, specific heat, system state density function, and fourth order Binder cumulants, the phase transitions in the Potts model with interactions J1<0 and J2<0 are shown to be found in value ranges of 0≤r<0.2 and 1.25≤r≤2.0. In an intermediate range of 0.2≤r≤1.0 the phase transition fails and the frustrations are revealed.
Bishop, R. F.; Li, P. H. Y.; Zinke, R.; Darradi, R.; Richter, J.; Farnell, D. J. J.; Schulenburg, J.
2017-04-01
We use the coupled cluster method (CCM) to study the ground-state properties and lowest-lying triplet excited state of the spin-half XXZ antiferromagnet on the square lattice. The CCM is applied to it to high orders of approximation by using an efficient computer code that has been written by us and which has been implemented to run on massively parallelized computer platforms. We are able therefore to present precise data for the basic quantities of this model over a wide range of values for the anisotropy parameter Δ in the range - 1 ≤ Δ 1) regimes, where Δ → ∞ represents the Ising limit. We present results for the ground-state energy, the sublattice magnetization, the zero-field transverse magnetic susceptibility, the spin stiffness, and the triplet spin gap. Our results provide a useful yardstick against which other approximate methods and/or experimental studies of relevant antiferromagnetic square-lattice compounds may now compare their own results. We also focus particular attention on the behaviour of these parameters for the easy-axis system in the vicinity of the isotropic Heisenberg point (Δ = 1) , where the model undergoes a phase transition from a gapped state (for Δ > 1) to a gapless state (for Δ ≤ 1), and compare our results there with those from spin-wave theory (SWT). Interestingly, the nature of the criticality at Δ = 1 for the present model with spins of spin quantum number s =1/2 that is revealed by our CCM results seems to differ qualitatively from that predicted by SWT, which becomes exact only for its near-classical large-s counterpart.
Han, Tianheng; Chu, Shaoyan; Lee, Young S
2012-04-13
We report thermodynamic measurements of the S=1/2 kagome lattice antiferromagnet ZnCu3(OH)6Cl2, a promising candidate system with a spin-liquid ground state. Using single crystal samples, the magnetic susceptibility both perpendicular and parallel to the kagome plane has been measured. A small, temperature-dependent anisotropy has been observed, where χ(z)/χ(p)>1 at high temperatures and χ(z)/χ(p)kagome Heisenberg antiferromagnet model to the experiments on ZnCu3(OH)6Cl2.
Dipolar order by disorder in the classical Heisenberg antiferromagnet on the kagome lattice.
Chern, Gia-Wei; Moessner, R
2013-02-15
Ever since the experiments which founded the field of highly frustrated magnetism, the kagome Heisenberg antiferromagnet has been the archetypical setting for the study of fluctuation induced exotic ordering. To this day the nature of its classical low-temperature state has remained a mystery: the nonlinear nature of the fluctuations around the exponentially numerous harmonically degenerate ground states has not permitted a controlled theory, while its complex energy landscape has precluded numerical simulations at low temperature, T. Here we present an efficient Monte Carlo algorithm which removes the latter obstacle. Our simulations detect a low-temperature regime in which correlations asymptote to a remarkably small value as T→0. Feeding these results into an effective model and analyzing the results in the framework of an appropriate field theory implies the presence of long-range dipolar spin order with a tripled unit cell.
Zhang, Yun; Lu, Haiyan; Zhu, Xiegang; Tan, Shiyong; Chen, Qiuyun; Feng, Wei; Xie, Donghua; Luo, Lizhu; Zhang, Wen; Lai, Xinchun; Donglai Feng Team; Huiqiu Yuan Team
One basic concept in heavy fermions systems is the entanglement of localized spin state and itinerant electron state. It can be tuned by two competitive intrinsic mechanisms, Kondo effect and Ruderman-Kittel-Kasuya-Yosida interaction, with external disturbances. The key issue regarding heavy fermions properties is how the two mechanisms work in the same phase region. To investigate the relation of the two mechanisms, the cubic antiferromagnetic heavy fermions compound CeIn3 was investigated by soft x-ray angle resolved photoemission spectroscopy. The hybridization between f electrons and conduction bands in the paramagnetic state was observed directly, providing compelling evidence for Kondo screening scenario and coexistence of two mechanisms. The hybridization strength shows slight and regular anisotropy in K space, implying that the two mechanisms are competitive and anisotropic. This work illuminates the concomitant and competitive relation between the two mechanisms and supplies some evidences for the anisotropic superconductivity of CeIn3
LIN ZhenQuan; KONG XiangMu; JIN JinShuang; YANG ZhanRu
2001-01-01
The Gaussian spin model with periodic interactions on the diamond-type hierarchical lattices is constructed by generalizing that with uniform interactions on translationally invariant lattices according to a class of substitution sequences. The Gaussian distribution constants and imposed external magnetic fields are also periodic depending on the periodic characteristic of the interaction bonds. The critical behaviors of this generalized Gaussian model in external magnetic fields are studied by the exact renormalization-group approach and spin rescaling method. The critical points and all the critical exponents are obtained. The critical behaviors are found to be determined by the Gaussian distribution constants and the fractal dimensions of the lattices. When all the Gaussian distribution constants are the same, the dependence of the critical exponents on the dimensions of the lattices is the same as that of the Gaussian model with uniform interactions on translationally invariant lattices.
Yarash K. Abuev; Albert B. Babaev; Pharkhat E. Esetov
2017-01-01
Objectives A computer simulation of the antiferromagnetic structures described by the three-vertex Potts model on a triangular lattice is performed, taking into account the antiferromagnetic exchange...
Neto, Minos A., E-mail: minos@pq.cnpq.br [Departamento de Fisica, Universidade Federal do Amazonas, 3000, Japiim, Manaus, 69077-000 AM (Brazil); Roberto Viana, J., E-mail: vianafisica@bol.com.br [Departamento de Fisica, Universidade Federal do Amazonas, 3000, Japiim, Manaus, 69077-000 AM (Brazil); Ricardo de Sousa, J., E-mail: jsousa@edu.ufam.br [Departamento de Fisica, Universidade Federal do Amazonas, 3000, Japiim, Manaus, 69077-000 AM (Brazil); National Institute of Science and Technology for Complex Systems, 3000, Japiim, Manaus, 69077-000 AM (Brazil)
2012-08-15
In this work we study the critical behavior of the quantum spin-1/2 anisotropic Heisenberg antiferromagnet in the presence of a longitudinal field on a body centered cubic (bcc) lattice as a function of temperature, anisotropy parameter ({Delta}) and magnetic field (H), where {Delta}=0 and 1 correspond the isotropic Heisenberg and Ising models, respectively. We use the framework of the differential operator technique in the effective-field theory with finite cluster of N=4 spins (EFT-4). The staggered m{sub s}=(m{sub A}-m{sub B})/2 and total m=(m{sub A}+m{sub B})/2 magnetizations are numerically calculated, where in the limit of m{sub s}{yields}0 the critical line T{sub N}(H,{Delta}) is obtained. The phase diagram in the T-H plane is discussed as a function of the parameter {Delta} for all values of H Element-Of [0,H{sub c}({Delta})], where H{sub c}({Delta}) correspond the critical field (T{sub N}=0). Special focus is given in the low temperature region, where a reentrant behavior is observed around of H=H{sub c}({Delta}){>=}H{sub c}({Delta}=1)=8J in the Ising limit, results in accordance with Monte Carlo simulation, and also was observed for all values of {Delta} Element-Of [0,1]. This reentrant behavior increases with increase of the anisotropy parameter {Delta}. In the limit of low field, our results for the Heisenberg limit are compared with series expansion values. - Highlights: Black-Right-Pointing-Pointer In the lat decade there has been a great interest in the physics of the quantum phase transition in spins system. Black-Right-Pointing-Pointer Effective-field theory in cluster with N=4 spins is generalized to treat the quantum spin-1/2 Heisenberg model. Black-Right-Pointing-Pointer We have obtained phase diagram at finite temperature for the quantum spin-1/2 antiferromagnet Heisenberg model as a bcc lattice.
Enhanced local lattice distortions with the antiferromagnetic transition in the multiferroic LuMnO3
Louca, Despina; Proffen, Thomas; Lee, Seung-Hun; Cheong, Sang-Wook
2009-03-01
The ferroelectric hexagonal manganite, LuMnO3, has been investigated via neutron scattering and the pair density function analysis to determine the nature of the local atomic distortions with the antiferromagnetic transition, TN, of the Mn ions. While in previously reported neutron diffraction data, it was shown that all atomic coordinates changed based on symmetry considerations with TN, we hereby show that it is the ferroelectric motion of the Lu ions coupled with O distortions that exhibits a strong temperature dependence below TN as reflected in the Lu-O bonds. This suggests an enhancement of the net electric polarization below TN. At the same time, the motion of the apical O1 and O2 ions distorts the MnO5 bipyramids, leading to more buckling of the ab-layers. However, the Mn ions do not appear to distort significantly away from their equilibrium position. The oxygen distortions induced with the spin reorientations below TN may be the cause for the Lu ion displacements through electrostatic interactions and this in turn produces coupling to the electric dipole moments.
Mazzucchi, Gabriel; Caballero-Benitez, Santiago F.; Mekhov, Igor B.
2016-08-01
Ultracold atomic systems offer a unique tool for understanding behavior of matter in the quantum degenerate regime, promising studies of a vast range of phenomena covering many disciplines from condensed matter to quantum information and particle physics. Coupling these systems to quantized light fields opens further possibilities of observing delicate effects typical of quantum optics in the context of strongly correlated systems. Measurement backaction is one of the most funda- mental manifestations of quantum mechanics and it is at the core of many famous quantum optics experiments. Here we show that quantum backaction of weak measurement can be used for tailoring long-range correlations of ultracold fermions, realizing quantum states with spatial modulations of the density and magnetization, thus overcoming usual requirement for a strong interatomic interactions. We propose detection schemes for implementing antiferromagnetic states and density waves. We demonstrate that such long-range correlations cannot be realized with local addressing, and they are a consequence of the competition between global but spatially structured backaction of weak quantum measurement and unitary dynamics of fermions.
Mazzucchi, Gabriel; Caballero-Benitez, Santiago F; Mekhov, Igor B
2016-08-11
Ultracold atomic systems offer a unique tool for understanding behavior of matter in the quantum degenerate regime, promising studies of a vast range of phenomena covering many disciplines from condensed matter to quantum information and particle physics. Coupling these systems to quantized light fields opens further possibilities of observing delicate effects typical of quantum optics in the context of strongly correlated systems. Measurement backaction is one of the most funda- mental manifestations of quantum mechanics and it is at the core of many famous quantum optics experiments. Here we show that quantum backaction of weak measurement can be used for tailoring long-range correlations of ultracold fermions, realizing quantum states with spatial modulations of the density and magnetization, thus overcoming usual requirement for a strong interatomic interactions. We propose detection schemes for implementing antiferromagnetic states and density waves. We demonstrate that such long-range correlations cannot be realized with local addressing, and they are a consequence of the competition between global but spatially structured backaction of weak quantum measurement and unitary dynamics of fermions.
The density of states for an antiferromagnetic Ising model on a triangular lattice
XIA Kai; YAO Xiao-yan; LIU Jun-ming
2007-01-01
The Wang-Landau algorithm is an efficient Monte Carlo approach to the density of states of a statistical mechanics system.The estimation of state density would allow the computation of thermodynamic properties of the system over the whole temperature range.We apply this sampling method to study the phase transitions in a triangular Ising model.The entropy of the lattice at zero temperature as well as other thermodynamic properties is computed.The calculated thermodynamic properties are explained in the context of the magnetic phase transition.
Wang, Wan-Sheng; Liu, Yuan-Chun; Xiang, Yuan-Yuan; Wang, Qiang-Hua
2016-07-01
We investigate the electronic instabilities in a kagome lattice with Rashba spin-orbital coupling by the unbiased singular-mode functional renormalization group. At the parent 1 /3 filling, the normal state is a quantum spin Hall system. Since the bottom of the conduction band is near the van Hove singularity, the electron-doped system is highly susceptible to competing orders upon electron interactions. The topological nature of the parent system enriches the complexity and novelty of such orders. We find 120∘-type intra-unit-cell antiferromagnetic order, f -wave superconductivity, and chiral p -wave superconductivity with increasing electron doping above the van Hove point. In both types of superconducting phases, there is a mixture of comparable spin singlet and triplet components because of the Rashba coupling. The chiral p -wave superconducting state is characterized by a Chern number Z =1 , supporting a branch of Weyl fermion states on each edge. The model bares close relevance to the so-called s d2 graphenes proposed recently.
Lattice distortion and stripelike antiferromagnetic order in Ca10(Pt3As8)(Fe2As2)5
Sapkota, Aashish [Ames Laboratory; Tucker, Gregory S [Ames Laboratory; Ramazanoglu, Mehmet [Ames Laboratory; Tian, Wei [Ames Laboratory; Ni, N [University of California; Cava, R J; McQueeney, Robert J [Princeton; Goldman, Alan I [Ames Laboratory; Kreyssig, Andreas [Ames Laboratory
2014-09-01
Ca10(Pt3As8)(Fe2As2)5 is the parent compound for a class of Fe-based high-temperature superconductors where superconductivity with transition temperatures up to 30 K can be introduced by partial element substitution. We present a combined high-resolution high-energy x-ray diffraction and elastic neutron scattering study on a Ca10(Pt3As8)(Fe2As2)5 single crystal. This study reveals the microscopic nature of two distinct and continuous phase transitions to be very similar to other Fe-based high-temperature superconductors: an orthorhombic distortion of the high-temperature tetragonal Fe-As lattice below TS=110(2) K followed by stripelike antiferromagnetic ordering of the Fe moments below TN=96(2) K. These findings demonstrate that major features of the Fe-based high-temperature superconductors are very robust against variations in chemical constitution as well as structural imperfection of the layers separating the Fe-As layers from each other and confirms that the Fe-As layers primarily determine the physics in this class of material.
Mi, Bin-Zhou
2017-02-01
The magnetic and thermodynamic properties of anisotropic frustrated spin-1 Heisenberg antiferromagnet on a body-centered cubic lattice for Néel phase (the region of weak frustration) are systematically investigated by use of the double-time Green's function method within the random phase approximation and the Anderson and Callen's decoupling. The zero-temperature sublattice magnetization and Néel temperature increase with spin anisotropy strength and single-ion anisotropy strength, and decrease with frustration strength. This indicates that quantum fluctuation is suppressed by spin anisotropy and single-ion anisotropy, by contrast, is strengthened by frustration. It is possible to tune the quantum fluctuations by the competition of anisotropy strength and frustration strength to change the ground state properties of magnetic materials. Although we find that both the spin anisotropy and the single-ion anisotropy suppress the quantum fluctuations, but their respective effects on the thermodynamic quantities, especially the internal energy and free energy, are different at zero temperature and finite temperature. Furthermore, when these two kinds of anisotropic coexist, the effect of the spin anisotropy on the sublattice magnetization and internal energy is larger than that of the single-ion anisotropy.
Large-N theory of the Sp(N) Heisenberg quantum antiferromagnet on an anisotropic triangular lattice
Chung, Chung-Hou; Marston, Brad
2000-03-01
The magnetic properties of the two-dimensional layered organic superconductors κ-(BEDT-TTF)_2X are modeled by a spin-1/2 Heisenberg quantum antiferromagnet on an anisotropic triangular lattice. The phase diagram is ascertained by means of a large-N expansion of the Sp(N) generalization of the physical SU(2) \\cong Sp(1) Heisenberg magnet.(S. Sachdev and N. Reed, Int. J. Mod. Phys. B5), 219 (1991). The phase diagram is presented in the two-dimensional parameter space of J_1/J_2, the ratio of the nearest to next-nearest neighbor Heisenberg exchange, and the ratio nb / N, which sets the strength of the quantum fluctuations. At large nb / N (equivalent to the large-spin limit of the physical SU(2) model) quantum effects are small, the ground states break global Sp(N) spin-rotational symmetry, and exhibit magnetic long-range-order (LRO). At small nb / N, however, quantum fluctuations overwhelm the tendency to order and there is only short-range magnetic order (SRO). The LRO and SRO phases can be further classified into two types depending on the size of the anisotropy: (i) ground states with commensurate, collinear, spin correlations; and (ii) ground states with incommensurate, coplanar, spin correlations. Finite-N corrections due to a Berry's phase term modify the character of the SRO phases, leading in the case of the commensurate state to spin-Peierls order and the confinement of spinons.
Babaev, A. B., E-mail: b-albert78@mail.ru; Magomedov, M. A.; Murtazaev, A. K. [Russian Academy of Sciences, Amirkhanov Institute of Physics, Dagestan Scientific Center (Russian Federation); Kassan-Ogly, F. A.; Proshkin, A. I. [Russian Academy of Sciences, Institute of Metal Physics, Ural Branch (Russian Federation)
2016-02-15
Phase transitions (PTs) and frustrations in two-dimensional structures described by a three-vertex antiferromagnetic Potts model on a triangular lattice are investigated by the Monte Carlo method with regard to nearest and next-nearest neighbors with interaction constants J{sub 1} and J{sub 2}, respectively. PTs in these models are analyzed for the ratio r = J{sub 2}/J{sub 1} of next-nearest to nearest exchange interaction constants in the interval |r| = 0–1.0. On the basis of the analysis of the low-temperature entropy, the density of states function of the system, and the fourth-order Binder cumulants, it is shown that a Potts model with interaction constants J{sub 1} < 0 and J{sub 2} < 0 exhibits a first-order PT in the range of 0 ⩽ r < 0.2, whereas, in the interval 0.2 ⩽ r ⩽ 1.0, frustrations arise in the system. At the same time, for J{sub 1} > 0 and J{sub 2} < 0, frustrations arise in the range 0.5 < |r| < 1.0, while, in the interval 0 ⩽ |r| ⩽ 1/3, the model exhibits a second-order PT.
Aoki, Dai; Paulsen, Carley; Kotegawa, Hisashi; Hardy, Frederic; Meingast, Christoph; Haen, Pierre; Boukahil, Mounir; Knafo, William; Ressouche, Eric; Raymond, Stephane; Flouquet, Jacques
2012-01-01
Doping Kondo lattice system CeRu2Si2 with Rh-8% (Ce(Ru0.92Rh0.08)2Si2) leads to drastic consequences due to the mismatch of the lattice parameters between CeRu2Si2 and CeRh2Si2. A large variety of experiments clarifies the unusual properties of the ground state induced by the magnetic field from longitudinal antiferromagnetic (AF) mode at H = 0 to polarized paramagnetic phase in very high magnetic field. The separation between AF phase, paramagnetic phase and polarized paramagnetic phase vary...
Hu, Wen-Jun; Gong, Shou-Shu; Sheng, D. N.
2016-08-01
By using Gutzwiller projected fermionic wave functions and variational Monte Carlo technique, we study the spin-1 /2 Heisenberg model with the first-neighbor (J1), second-neighbor (J2), and additional scalar chiral interaction JχSi.(Sj×Sk) on the triangular lattice. In the nonmagnetic phase of the J1-J2 triangular model with 0.08 ≲J2/J1≲0.16 , recent density-matrix renormalization group (DMRG) studies [Zhu and White, Phys. Rev. B 92, 041105(R) (2015), 10.1103/PhysRevB.92.041105 and Hu, Gong, Zhu, and Sheng, Phys. Rev. B 92, 140403(R) (2015), 10.1103/PhysRevB.92.140403] find a possible gapped spin liquid with the signal of a competition between a chiral and a Z2 spin liquid. Motivated by the DMRG results, we consider the chiral interaction JχSi.(Sj×Sk) as a perturbation for this nonmagnetic phase. We find that with growing Jχ, the gapless U(1) Dirac spin liquid, which has the best variational energy for Jχ=0 , exhibits the energy instability towards a gapped spin liquid with nontrivial magnetic fluxes and nonzero chiral order. We calculate topological Chern number and ground-state degeneracy, both of which identify this flux state as the chiral spin liquid with fractionalized Chern number C =1 /2 and twofold topological degeneracy. Our results indicate a positive direction to stabilize a chiral spin liquid near the nonmagnetic phase of the J1-J2 triangular model.
Honda, Zentaro; Kodama, Takafumi; Hagiwara, Masayuki; Kida, Takanori; Okutani, Akira; Sakai, Masamichi; Fukuda, Takeshi; Kamata, Norihiko
2016-09-01
We report on the syntheses, crystal structures, and magnetic properties of a series of transition metal coordination polymers M2(pymca)3(ClO4), (pymca = pyrimidine-2-carboxylic acid, M = Fe (1), Co (2), and Ni (3)). These compounds are found to crystallize in a trigonal crystal system, space group P31m, with the lattice constants a = 9.727 Å and c = 5.996 Å for 1, a = 9.608 Å and c = 5.996 Å for 2, and a = 9.477 Å and c = 5.958 Å for 3 at room temperature. In these compounds, each pymca ligand connects to two M2+ ions, forming a honeycomb network in the ab plane. The temperature dependences of magnetic susceptibilities in these compounds show broad maxima, indicating antiferromagnetic interactions within two-dimensional honeycomb layers. We also observed an antiferromagnetic phase transition at low temperatures by magnetic susceptibility and heat capacity measurements. From the crystal structures and magnetic properties, we conclude that the compounds 1, 2, and 3 are good realizations of honeycomb-lattice antiferromagnets.
Antezza, Mauro; Castin, Yvan
2013-09-01
We study the effects of finite size and of vacancies on the photonic band gap recently predicted for an atomic diamond lattice. Close to a Jg=0→Je=1 atomic transition, and for atomic lattices containing up to N≈3×104 atoms, we show how the density of states can be affected by both the shape of the system and the possible presence of a fraction of unoccupied lattice sites. We numerically predict and theoretically explain the presence of shape-induced border states and of vacancy-induced localized states appearing in the gap. We also investigate the penetration depth of the electromagnetic field which we compare to the case of an infinite system.
Henriques, M. S.; Gorbunov, D. I.; Kriegner, D.; Vališka, M.; Andreev, A. V.; Matěj, Z.
2016-02-01
Structural changes through the first-order paramagnetic-antiferromagnetic phase transition of Dy3Ru4Al12 at 7 K have been studied by means of X-ray diffraction and thermal expansion measurements. The compound crystallizes in a hexagonal crystal structure of Gd3Ru4Al12 type (P63/mmc space group), and no structural phase transition has been found in the temperature interval between 2.5 and 300 K. Nevertheless, due to the spin-lattice coupling the crystal volume undergoes a small orthorhombic distortion of the order of 2×10-5 as the compound enters the antiferromagnetic state. We propose that the first-order phase transition is not driven by the structural changes but rather by the exchange interactions present in the system.
Shore, Joel D.; Thurston, George M.
2015-12-01
We report a charge-patterning phase transition on two-dimensional square lattices of titratable sites, here regarded as protonation sites, placed in a low-dielectric medium just below the planar interface between this medium and a salt solution. We calculate the work-of-charging matrix of the lattice with use of a linear Debye-Hückel model, as input to a grand-canonical partition function for the distribution of occupancy patterns. For a large range of parameter values, this model exhibits an approximate inverse cubic power-law decrease of the voltage produced by an individual charge, as a function of its in-lattice separation from neighboring titratable sites. Thus, the charge coupling voltage biases the local probabilities of proton binding as a function of the occupancy of sites for many neighbors beyond the nearest ones. We find that even in the presence of these longer-range interactions, the site couplings give rise to a phase transition in which the site occupancies exhibit an alternating, checkerboard pattern that is an analog of antiferromagnetic ordering. The overall strength W of this canonical charge coupling voltage, per unit charge, is a function of the Debye length, the charge depth, the Bjerrum length, and the dielectric coefficients of the medium and the solvent. The alternating occupancy transition occurs above a curve of thermodynamic critical points in the (p H-p K ,W ) plane, the curve representing a charge-regulation analog of variation of the Néel temperature of an Ising antiferromagnet as a function of an applied, uniform magnetic field. The analog of a uniform magnetic field in the antiferromagnet problem is a combination of p H-p K and W , and 1 /W is the analog of the temperature in the antiferromagnet problem. We use Monte Carlo simulations to study the occupancy patterns of the titratable sites, including interactions out to the 37th nearest-neighbor category (a distance of √{74 } lattice constants), first validating simulations
Lima, L. S.
2017-02-01
We have used the Dirac's massless quasi-particles together with the Kubo's formula to study the spin transport by electrons in the graphene monolayer. We have calculated the electric conductivity and verified the behavior of the AC and DC currents of this system, that is a relativistic electron plasma. Our results show that the AC conductivity tends to infinity in the limit ω → 0 , similar to the behavior obtained for the spin transport in the two-dimensional frustrated antiferromagnet in the honeycomb lattice. We have made a diagrammatic expansion for the Green's function and we have not gotten significative change in the results.
Aoki, Dai; Paulsen, Carley; Kotegawa, Hisashi; Hardy, Frédéric; Meingast, Christoph; Haen, Pierre; Boukahil, Mounir; Knafo, William; Ressouche, Eric; Raymond, Stephane; Flouquet, Jacques
2012-03-01
Doping Kondo lattice system CeRu2Si2 with Rh-8% (Ce(Ru0.92Rh0.08)2Si2) leads to drastic consequences due to the mismatch of the lattice parameters between CeRu2Si2 and CeRh2Si2. A large variety of experiments clarifies the unusual properties of the ground state induced by the magnetic field from longitudinal antiferromagnetic (AF) mode at H=0 to polarized paramagnetic phase in very high magnetic field. The separation between AF phase, paramagnetic phase and polarized paramagnetic phase varying with temperature, magnetic field and pressure is discussed on the basis of the experiments down to very low temperature. Similarities and differences between Rh and La substituted alloys are discussed with emphasis on the competition between transverse and longitudinal AF modes, and ferromagnetic fluctuations.
Huang, Ran; Gujrati, Purushottam D.
2017-01-01
An inhomogeneous 2-dimensional recursive lattice formed by planar elements has been designed to investigate the thermodynamics of Ising spin system on the surface/thin film. The lattice is constructed as a hybrid of partial Husimi square lattice representing the bulk and 1D single bonds representing the surface. Exact calculations can be achieved with the recursive property of the lattice. The model has an anti-ferromagnetic interaction to give rise to an ordered phase identified as crystal, and a solution with higher energy to represent the amorphous/metastable phase. Free energy and entropy of the ideal crystal and supercooled liquid state of the model on the surface are calculated by the partial partition function. By analyzing the free energies and entropies of the crystal and supercooled liquid state, we are able to identify the melting and ideal glass transition on the surface. The results show that due to the variation of coordination number, the transition temperatures on the surface decrease significantly compared to the bulk system. Our calculation qualitatively agrees with both experimental and simulation works on the thermodynamics of surfaces and thin films conducted by others. Interactions between particles farther than the nearest neighbor distance are taken into consideration, and their effects are investigated. Supported by the National Natural Science Foundation of China under Grant No. 11505110, the Shanghai Pujiang Talent Program under Grant No. 16PJ1431900, and the China Postdoctoral Science Foundation under Grant No. 2016M591666
L. Gálisová
2011-03-01
Full Text Available Phase transitions of the mixed spin-1/2 and spin-1 Ising-Heisenberg model on several decorated planar lattices consisting of interconnected diamonds are investigated within the framework of the generalized decoration-iteration transformation. The main attention is paid to the systematic study of the finite-temperature phase diagrams in dependence on the lattice topology. The critical behaviour of the hybrid quantum-classical Ising-Heisenberg model is compared with the relevant behaviour of its semi-classical Ising analogue. It is shown that both models on diamond-like decorated planar lattices exhibit a striking critical behaviour including reentrant phase transitions. The higher the lattice coordination number is, the more pronounced reentrance may be detected.
Nunes, Wagner A; de Sousa, J Ricardo; Viana, J Roberto; Richter, J
2010-04-14
The ground state phase diagram of the quantum spin-1/2 Heisenberg antiferromagnet in the presence of nearest-neighbor (J(1)) and next-nearest-neighbor (J(2)) interactions (J(1)-J(2) model) on a stacked square lattice, where we introduce an interlayer coupling through nearest-neighbor bonds of strength J(), is studied within the framework of the differential operator technique. The Hamiltonian is solved by effective-field theory in a cluster with N=4 spins (EFT-4). We obtain the sublattice magnetization m(A) for the ordered phases: antiferromagnetic (AF) and collinear (CAF-collinear antiferromagnetic). We propose a functional for the free energy Ψ(μ)(m(μ)) (μ=A, B) to obtain the phase diagram in the λ-α plane, where λ=J()/J(1) and α=J(2)/J(1). Depending on the values of λ and α, we found different ordered states (AF and CAF) and a disordered state (quantum paramagnetic (QP)). For an intermediate region α(1c)(λ) α(2c)(λ), and below λ(1), we have the AF and CAF semi-classically ordered states, respectively. At α=α(1c)(λ) a second-order transition between the AF and QP states occurs and at α=α(2c)(λ) a first-order transition between the AF and CAF phases takes place. The boundaries between these ordered phases merge at the critical end point CEP≡(λ(1), α(c)), where α(c)≈0.56. Above this CEP there is again a direct first-order transition between the AF and CAF phases, with a behavior described by the point α(c) independent of λ ≥ λ(1).
Hu, Wen-Jun; Gong, Shou-Shu; Becca, Federico; Sheng, D. N.
2015-11-01
By using the variational Monte Carlo technique, we study the spin-1/2 XXZ antiferromagnetic model (with easy-plane anisotropy) on the kagome lattice. A class of Gutzwiller projected fermionic states with a spin Jastrow factor is considered to describe either spin liquids [with U (1 ) or Z2 symmetry] or magnetically ordered phases [with q =(0 ,0 ) or q =(4 π /3 ,0 ) ]. We find that the magnetic states are not stable in the thermodynamic limit. Moreover, there is no energy gain to break the gauge symmetry from U (1 ) to Z2 within the spin-liquid states, as previously found in the Heisenberg model. The best variational wave function is therefore the U (1 ) Dirac state, supplemented by the spin Jastrow factor. Furthermore, a vanishing S =2 spin gap is obtained at the variational level, in the whole regime from the X Y to the Heisenberg model.
Zhu, Rengui, E-mail: rgzhu@mail.ahnu.edu.cn; Hu, Gangsan
2013-06-15
A frustrated Heisenberg model on a stacked square lattice in a striped antiferromagnetic spin order is studied by the Green's function approach. Besides the intra- and inter-layer exchange couplings, the single-ion anisotropy (J{sub s}) is also considered. The expressions of the spin spectrum gap (Δ), the transition temperature (T{sub N}) and the zero-temperature average spin (〈S{sup z}〉{sub 0}) are derived analytically. Their dependences on the single-ion anisotropy are investigated. We find they are all increasing functions of J{sub s}. We make a further estimation of the magnitude of J{sub s} according to the experimental temperature T{sub N}=138K of the pure compound LaFeAsO.
Pires, A.S.T. [Departamento de Fisica, Universidade Federal de Minas Gerais, Belo Horizonte, MG, CP 702, 30123-970 (Brazil); Lapa, R.S., E-mail: rodrigophc@gmail.com [Departamento de Fisica, Universidade Federal de Minas Gerais, Belo Horizonte, MG, CP 702, 30123-970 (Brazil)
2013-08-15
We study the disordered phase of the J{sub 1}–J{sub 2} frustrated Heisenberg antiferromagnet with spin S=1 on a square lattice using a SU(3) Schwinger boson representation. In the approximation of Bose condensation and in a mean-field treatment of the four-operator terms, we calculate the gap as a function of J{sub 1}/J{sub 2}, and the quadrupole static structure factor at zero temperature. Our results indicate the existence of a nematic state in the paramagnetic phase. - Highlights: ► The disordered phase is studied. ► The energy gap in the paramagnetic phase is calculated. ► The static spin structure factor is calculated. ► The static quadrupole structure factor is calculated. ► The ground state energy is calculated.
Susuki, Takuya; Kurita, Nobuyuki; Tanaka, Takuya; Nojiri, Hiroyuki; Matsuo, Akira; Kindo, Koichi; Tanaka, Hidekazu
2013-06-28
We have performed high-field magnetization and electronic spin resonance (ESR) measurements on Ba3CoSb2O9 single crystals, which approximates the two-dimensional (2D) S=1/2 triangular-lattice Heisenberg antiferromagnet. For an applied magnetic field H parallel to the ab plane, the entire magnetization curve including the plateau at one-third of the saturation magnetization (Ms) is in excellent agreement with the results of theoretical calculations except a small step anomaly near (3/5)Ms, indicative of a theoretically undiscovered quantum phase transition. However, for H∥c, the magnetization curve exhibits a cusp near Ms/3 owing to the weak easy-plane anisotropy and the 2D quantum fluctuation. From a detailed analysis of the collective ESR modes observed in the ordered state, combined with the magnetization process, we have determined all the magnetic parameters including the interlayer and anisotropic exchange interactions.
Babkevich, P.; Katukuri, Vamshi M.; Fâk, B.; Rols, S.; Fennell, T.; Pajić, D.; Tanaka, H.; Pardini, T.; Singh, R. R. P.; Mitrushchenkov, A.; Yazyev, O. V.; Rønnow, H. M.
2016-12-01
Sr2 CuTeO6 presents an opportunity for exploring low-dimensional magnetism on a square lattice of S =1 /2 Cu2 + ions. We employ ab initio multireference configuration interaction calculations to unravel the Cu2 + electronic structure and to evaluate exchange interactions in Sr2 CuTeO6 . The latter results are validated by inelastic neutron scattering using linear spin-wave theory and series-expansion corrections for quantum effects to extract true coupling parameters. Using this methodology, which is quite general, we demonstrate that Sr2 CuTeO6 is an almost ideal realization of a nearest-neighbor Heisenberg antiferromagnet but with relatively weak coupling of 7.18(5) meV.
Matan, K., E-mail: kmatan@issp.u-tokyo.ac.j [Department of Physics, Massachusetts Institute of Technology, Cambridge, MA 02139 (United States); Helton, J.S. [Department of Physics, Massachusetts Institute of Technology, Cambridge, MA 02139 (United States); Grohol, D. [The Dow Chemical Company, Core R and D, Midland, MI 48674 (United States); Nocera, D.G. [Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA 02139 (United States); Wakimoto, S.; Kakurai, K. [Quantum Beam Science Directorate, Japanese Atomic Energy Agency, 2-4 Shirakata Shirane, Tokai, Naka, Ibaraki 319-1195 (Japan); Lee, Y.S. [Department of Physics, Massachusetts Institute of Technology, Cambridge, MA 02139 (United States)
2009-09-01
We report polarized neutron scattering studies of spin-wave excitations and spin fluctuations in the S=5/2 kagome{sup '} lattice antiferromagnet KFe{sub 3}(OH){sub 6}(SO{sub 4}){sub 2} (jarosite). Inelastic polarized neutron scattering measurements at 10 K on a single crystal sample reveal two spin gaps, associated with in-plane and out-of-plane excitations. The polarization analysis of quasi-elastic scattering at 67 K shows in-plane spin fluctuations with XY symmetry, consistent with the disappearance of the in-plane gap above the Neel temperature T{sub N}=65K. Our results suggest that jarosite is a promising candidate for studying the 2D XY universality class in magnetic systems.
Majumdar, Kingshuk; Datta, Trinanjan
2009-10-07
At zero temperature the sublattice magnetization of the quantum spin- 1/2 Heisenberg antiferromagnet on a body-centered cubic lattice with competing first and second neighbor exchange (J(1) and J(2)) is investigated using the non-linear spin wave theory. The zero temperature phases of the model consist of a two sublattice Néel phase for small J(2) (AF(1)) and a collinear phase at large J(2) (AF(2)). We show that quartic corrections due to spin wave interactions enhance the sublattice magnetization in both the AF(1) and the AF(2) phase. The magnetization corrections are prominent near the classical transition point of the model and in the J(2)>J(1) regime. The ground state energy with quartic interactions is also calculated. It is found that up to quartic corrections the first order phase transition (previously observed in this model) between the AF(1) and the AF(2) phase survives.
Spin dynamics and spin freezing in the triangular lattice antiferromagnets FeGa2S4 and NiGa2S4
Zhao, Songrui; Dalmas de Réotier, P.; Yaouanc, A.; MacLaughlin, D. E.; Mackie, J. M.; Bernal, O. O.; Nambu, Y.; Higo, T.; Nakatsuji, S.
2012-08-01
Magnetic susceptibility and muon spin relaxation (μSR) experiments have been carried out on the quasi-2D triangular-lattice spin S=2 antiferromagnet FeGa2S4. The μSR data indicate a sharp onset of a frozen or nearly frozen spin state at T*=31(2) K, twice the spin-glass-like freezing temperature Tf=16(1) K. The susceptibility becomes field dependent below T*, but no sharp anomaly is observed in any bulk property. A similar transition is observed in μSR data from the spin-1 isomorph NiGa2S4. In both compounds the dynamic muon spin relaxation rate λd(T) above T* agrees well with a calculation of spin-lattice relaxation by Chubukov, Sachdev, and Senthil in the renormalized classical regime of a 2D frustrated quantum antiferromagnet. There is no firm evidence for other mechanisms. At low temperatures, λd(T) becomes temperature independent in both compounds, indicating persistence of spin dynamics. Scaling of λd(T) between the two compounds is observed from ˜Tf to ˜1.5T*. Although the μSR data by themselves cannot exclude a truly static spin component below T*, together with the susceptibility data they are consistent with a slowly fluctuating “spin gel” regime between Tf and T*. Such a regime and the absence of a divergence in λd(T) at T* are features of two unconventional mechanisms: (1) binding/unbinding of Z2 vortex excitations, and (2) impurity spins in a nonmagnetic spin-nematic ground state. The absence of a sharp anomaly or history dependence at T* in the susceptibility of FeGa2S4, and the weakness of such phenomena in NiGa2S4, strongly suggest transitions to low-temperature phases with unconventional dynamics.
Bera, A. K.; Yusuf, S. M.; Kumar, Amit; Ritter, C.
2017-03-01
The crystal structure, magnetic ground state, and the temperature-dependent microscopic spin-spin correlations of the frustrated honeycomb lattice antiferromagnet N a2C o2Te O6 have been investigated by powder neutron diffraction. A long-range antiferromagnetic (AFM) ordering has been found below TN˜24.8 K . The magnetic ground state, determined to be zigzag antiferromagnetic and characterized by a propagation vector k =(1 /2 0 0 ) , occurs due to the competing exchange interactions up to third-nearest neighbors within the honeycomb lattice. The exceptional existence of a limited magnetic correlation length along the c axis (perpendicular to the honeycomb layers in the a b planes) has been found even at 1.8 K, well below the TN˜24.8 K . The observed limited correlation along the c axis is explained by the disorder distribution of the Na ions within the intermediate layers between honeycomb planes. The reduced ordered moments mCo (1 )=2.77 (3 ) μB/C o2 + and mCo (2 )=2.45 (2 ) μB/C o2 + at 1.8 K reflect the persistence of spin fluctuations in the ordered state. Above TN˜24.8 K , the presence of short-range magnetic correlations, manifested by broad diffuse magnetic peaks in the diffraction patterns, has been found. Reverse Monte Carlo analysis of the experimental diffuse magnetic scattering data reveals that the spin correlations are mainly confined within the two-dimensional honeycomb layers (a b plane) with a correlation length of ˜12 Å at 25 K. The nature of the spin arrangements is found to be similar in both the short-range and long-range ordered magnetic states. This implies that the short-range correlation grows with decreasing temperature and leads to the zigzag AFM ordering at T ≤TN . The present study provides a comprehensive picture of the magnetic correlations over the temperature range above and below the TN and their relation to the crystal structure. The role of intermediate soft Na layers on the magnetic coupling between honeycomb planes is
Capponi, Sylvain
2017-01-01
We present numerical evidence that the spin-1/2 Heisenberg model on the two-dimensional checkerboard lattice exhibits several magnetization plateaus for m =0 , 1 /4 , 1 /2 , and 3 /4 , where m is the magnetization normalized by its saturation value. These incompressible states correspond to somewhat similar valence-bond crystal phases that break lattice symmetries, though they are different from the already established plaquette phase for m =0 . Our results are based on exact diagonalization as well as density-matrix renormalization-group large-scale simulations and interpreted in terms of simple parameter-free trial wave functions.
YAO Xiao-yan; LI Peng-lei; DONG Shuai; LIU Jun-ming
2007-01-01
A three-dimensional Ising-like model doped with anti-ferromagnetic (AFM) bonds is proposed to investigate the magnetic properties of a doped triangular spin-chain system by using a Monte-Carlo simulation. The simulated results indicate that a steplike magnetization behavior is very sensitive to the concentration of AFM bonds. A low concentration of AFM bonds can suppress the stepwise behavior considerably, in accordance with doping experiments on Ca3Co206. The analysis of spin snapshots demonstrates that the AFM bond doping not only breaks the ferromagnetic ordered linear spin chains along the hexagonal c-axis but also has a great influence upon the spin configuration in the ab-plane.
Antiferromagnetic spintronics.
Jungwirth, T; Marti, X; Wadley, P; Wunderlich, J
2016-03-01
Antiferromagnetic materials are internally magnetic, but the direction of their ordered microscopic moments alternates between individual atomic sites. The resulting zero net magnetic moment makes magnetism in antiferromagnets externally invisible. This implies that information stored in antiferromagnetic moments would be invisible to common magnetic probes, insensitive to disturbing magnetic fields, and the antiferromagnetic element would not magnetically affect its neighbours, regardless of how densely the elements are arranged in the device. The intrinsic high frequencies of antiferromagnetic dynamics represent another property that makes antiferromagnets distinct from ferromagnets. Among the outstanding questions is how to manipulate and detect the magnetic state of an antiferromagnet efficiently. In this Review we focus on recent works that have addressed this question. The field of antiferromagnetic spintronics can also be viewed from the general perspectives of spin transport, magnetic textures and dynamics, and materials research. We briefly mention this broader context, together with an outlook of future research and applications of antiferromagnetic spintronics.
Magnetic phases of the quasi-two-dimensional antiferromagnet CuCrO2 on a triangular lattice
Sakhratov, Yu. A.; Svistov, L. E.; Kuhns, P. L.; Zhou, H. D.; Reyes, A. P.
2016-09-01
We have carried out Cu,6563 NMR spectra measurements in a magnetic field up to about 45 T on a single crystal of a multiferroic triangular antiferromagnet CuCrO2. The measurements were performed for magnetic fields aligned along the crystal c axis. Field and temperature evolution of the spectral shape demonstrates a number of phase transitions. It was found that the 3D magnetic ordering takes place in the low field range (H ≲15 T). At higher fields magnetic structures form within individual triangular planes whereas the spin directions of the magnetic ions from neighboring planes are not correlated. It is established that the 2D-3D transition is hysteretic in field and temperature. Line-shape analysis reveals several possible magnetic structures existing within individual planes for different phases of CuCrO2. Within certain regions on the magnetic H -T phase diagram of CuCrO2 a 3D magnetic ordering with tensor order parameter is expected.
Okubo, Susumu; Nakata, Ryohei; Ikeda, Shohei; Takahashi, Naoki; Sakurai, Takahiro; Zhang, Wei-Min; Ohta, Hitoshi; Shimokawa, Tokuro; Sakai, Tôru; Okuta, Koji; Hara, Shigeo; Sato, Hirohiko
2017-02-01
A single-crystal S = 3/2 perfect kagome lattice antiferromagnet, KCr3(OH)6(SO4)2 (Cr-jarosite), has been studied by X-band and high-frequency electron spin resonance (ESR). The g-values perpendicular to the kagome plane (c-axis) and in the plane were determined to be gc = 1.9704 ± 0.0002 and gξ = 1.9720 ± 0.0003, respectively, by high-frequency ESR observed at 265 K. Antiferromagnetic resonances (AFMRs) with an antiferromagnetic gap of 120 GHz were observed at 1.9 K, which is below TN = 4.5 K. The analysis of AFMR modes using the conventional molecular field theory gave dp = 0.27 K and dz = 0.07 K, where dp and dz are in-plane and out-of-plane components of d vector of the Dzyaloshinsky-Moriya (DM) interaction, respectively. On the basis of these results and the exchange interaction of J = 6.15 K estimated by Okuta et al., the ground state of Cr-jarosite was discussed in connection with the Monte Carlo simulation results with classical Heisenberg spins on the kagome lattice by Elhajal et al. Finally, the angular dependence of the linewidth and lineshape observed at 296 K by X-band ESR showed the typical behavior of a two-dimensional Heisenberg antiferromagnet, suggesting the good two-dimensionality of Cr-jarosite.
Yoshida, Hiroyuki; Noguchi, Naoya; Matsushita, Yoshitaka; Ishii, Yuto; Ihara, Yoshihiko; Oda, Migaku; Okabe, Hirotaka; Yamashita, Satoshi; Nakazawa, Yasuhiro; Takata, Atsushi; Kida, Takanori; Narumi, Yasuo; Hagiwara, Masayuki
2017-03-01
We have succeeded in preparing single crystals of CaCu3(OH)6Cl2 • 0.6H2O, a candidate for the S = 1/2 Kagome lattice antiferromagnet. Magnetic properties of the compound are dominated by the nearest neighbor antiferromagnetic interaction J1, and the next nearest neighbor ferromagnetic J2 and an antiferromagnetic Jd across a hexagon, which is different from related compounds Kapellasite and Haydeeite with ferromagnetic J1. Magnetic susceptibility exhibits a sudden increase below 13 K and a cusp anomaly at T* = 7.2 K in the ab-plane, whereas only a moderate enhancement is observed below T* along the c-axis. A tiny peak detected in heat capacity at T* indicates the occurrence of a magnetic phase transition. The low temperature magnetic heat capacity was reproduced by assuming a two-dimensional spin-wave component and a temperature-linear term. The spin-wave contribution suggests a magnon excitation in a short-range ordered region, whereas the relatively large T-linear term 5.9 mJ/(Cu-mol·K2) at H = 0 T of this insulating compound suggests the existence of an unusual quasi-particle excitation below T*. They apparently reveal the unconventionality of the ground state of this S = 1/2 Kagome lattice antiferromagnet.
Huang, Yi-Zhen; Xi, Bin; Chen, Xi; Li, Wei; Wang, Zheng-Chuan; Su, Gang
2016-06-01
The quantum phase transition, scaling behaviors, and thermodynamics in the spin-1/2 quantum Heisenberg model with antiferromagnetic coupling J >0 in the armchair direction and ferromagnetic interaction J'Monte Carlo method. By calculating the Binder ratio Q2 and spin stiffness ρ in two directions for various coupling ratios α =J'/J under different lattice sizes, we found that a quantum phase transition from the dimerized phase to the stripe phase occurs at the quantum critical point αc=-0.93 . Through the finite-size scaling analysis on Q2, ρx, and ρy, we determined the critical exponent related to the correlation length ν to be 0.7212(8), implying that this transition falls into a classical Heisenberg O(3) universality. A zero magnetization plateau is observed in the dimerized phase, whose width decreases with increasing α . A phase diagram in the coupling ratio α -magnetic field h plane is obtained, where four phases, including dimerized, stripe, canted stripe, and polarized, are identified. It is also unveiled that the temperature dependence of the specific heat C (T ) for different α 's intersects precisely at one point, similar to that of liquid 3He under different pressures and several magnetic compounds under various magnetic fields. The scaling behaviors of Q2, ρ , and C (T ) are carefully analyzed. The susceptibility is compared with the experimental data to give the magnetic parameters of both compounds.
Kumar, Krishna; Changlani, Hitesh J.; Clark, Bryan K.; Fradkin, Eduardo
2016-10-01
We perform an exact-diagonalization study of the spin-1/2 XXZ Heisenberg antiferromagnet on the kagome lattice at finite magnetization m =2/3 with an emphasis on the X Y point (Jz=0 ) and in the presence of a small chiral term. Recent analytic work by Kumar et al. [K. Kumar, K. Sun, and E. Fradkin, Phys. Rev. B 90, 174409 (2014), 10.1103/PhysRevB.90.174409] on the same model, using a newly developed flux attachment transformation, predicts a plateau at this value of the magnetization described by a chiral spin liquid (CSL) with a spin Hall conductance of σx y=1/2 . Such a state is topological in nature, has a ground-state degeneracy, and exhibits fractional excitations. We analyze the degeneracy structure in the low-energy manifold, identify the candidate topological states, and use them to compute the modular matrices and Chern numbers, all of which strongly agree with expected theoretical behavior for the σx y=1/2 CSL. In the limit of zero chirality, we find on most (not all) clusters that the topological invariants are still those of a CSL.
Canted antiferromagnetism in KNi3[PO3(F,OH)]2[PO2(OH)2]F2 with a stair-case Kagomé lattice
Liu, Li-Chen; Ren, Wei-Jian; Huang, Ya-Xi; Pan, Yuanming; Mi, Jin-Xiao
2017-10-01
A new nickel phosphate KNi3[PO3(F,OH)]2[PO2(OH)2]F2 has been synthesized using a modified hydrothermal method. Structural characterizations show that it adopts a 3D framework structure with 2D layers of Ni octahedra in a stair-case Kagomé lattice. The Ni2 octahedron at the inversion center shares two trans-faces with Ni1 octahedra to form a linear trimer (Ni3O8F6) as the basic structural unit. The Ni-trimers are linked between themselves by sharing F-corners and to [PO3(F,OH)] tetrahedral groups by sharing O-corners to form 2D stair-case Kagomé layers, which are parallel to the (100) plane and are stacked along the a-axis. Successive Kagomé layers are combined together by [PO2(OH)2] tetrahedral groups and interstice cations K+. Magnetic measurements reveal that KNi3[PO3(F,OH)]2[PO2(OH)2]F2 exhibits a canted antiferromagnetic ordering with a ferromagnetic component at low temperatures.
Wang, Guangmei [Ruhr-Universitat Bochum; Valldor, Martin [Max Plank Institute for Chemical Physics of Solids, Dresden, Germany; Mallick, Bert [Ruhr Universitat Bochum; Mudring, Anja-Verena [Ames Laboratory
2014-01-01
Four open-framework transition-metal phosphates; (NH4)2Co3(HPO4)2F4 (1), (NH4)Co3(HPO4)2(H2PO4)F2 (2), KCo3(HPO4)2(H2PO4)F2 (3), and KFe3(HPO4)2(H2PO4)F2 (4); are prepared by ionothermal synthesis using pyridinium hexafluorophosphate as the ionic liquid. Single-crystal X-ray diffraction analyses reveal that the four compounds contain cobalt/iron–oxygen/fluoride layers with Kagomé topology composed of interlinked face-sharing MO3F3/MO4F2 octahedra. PO3OH pseudo-tetrahedral groups augment the [M3O6F4] (1)/[M3O8F2] layers on both sides to give M3(HPO4)2F4 (1) and M3(HPO4)2F2 (2–4) layers. These layers are stacked along the a axis in a sequence AA…, resulting in the formation of a layer structure for (NH4)2Co3(HPO4)2F4(1). In NH4Co3(HPO4)2(H2PO4)F2 and KM3(HPO4)2(H2PO4)F2, the M3(HPO4)2F2 layers are stacked along the a axis in a sequence AAi… and are connected by [PO3(OH)] tetrahedra, giving rise to a 3-D open framework structure with 10-ring channels along the [001] direction. The negative charges of the inorganic framework are balanced by K+/NH4+ ions located within the channels. The magnetic transition metal cations themselves form layers with stair-case Kagomé topology. Magnetic susceptibility and magnetization measurements reveal that all four compounds exhibit a canted anti-ferromagnetic ground state (Tc = 10 or 13 K for Co and Tc = 27 K for Fe) with different canting angles. The full orbital moment is observed for both Co2+ and Fe2+.
Shimokawa, Tokuro; Watanabe, Ken; Kawamura, Hikaru
2015-10-01
Inspired by the recent theoretical suggestion that the random-bond S =1 /2 antiferromagnetic Heisenberg model on the triangular and the kagome lattices might exhibit a randomness-induced quantum spin liquid (QSL) behavior when the strength of the randomness exceeds a critical value, and that this "random-singlet state" might be relevant to the QSL behaviors experimentally observed in triangular organic salts κ -(ET) 2Cu2(CN) 3 and EtMe3Sb [Pd(dmit)2] 2 and in kagome herbertsmithite ZnCu3(OH) 6Cl2 , we further investigate the nature of the static and the dynamical spin correlations of these models. We compute the static and the dynamical spin structure factors, S (q ) and S (q ,ω ) , by means of an exact diagonalization method. In both triangular and kagome models, the computed S (q ,ω ) in the random-singlet state depends on the wave vector q only weakly, robustly exhibiting gapless behaviors accompanied by the broad distribution extending to higher energy ω . Especially in the strongly random kagome model, S (q ,ω ) hardly depends on q , and exhibits an almost flat distribution for a wide range of ω , together with a ω =0 peak. These features agree semiquantitatively with the recent neutron-scattering data on a single-crystal herbertsmithite. Furthermore, the computed magnetization curve agrees almost quantitatively with the experimental one recently measured on a single-crystal herbertsmithite. These results suggest that the QSL state observed in herbertsmithite might indeed be the randomness-induced QSL state, i.e., the random-singlet state.
Electrical switching of an antiferromagnet.
Wadley, P; Howells, B; Železný, J; Andrews, C; Hills, V; Campion, R P; Novák, V; Olejník, K; Maccherozzi, F; Dhesi, S S; Martin, S Y; Wagner, T; Wunderlich, J; Freimuth, F; Mokrousov, Y; Kuneš, J; Chauhan, J S; Grzybowski, M J; Rushforth, A W; Edmonds, K W; Gallagher, B L; Jungwirth, T
2016-02-05
Antiferromagnets are hard to control by external magnetic fields because of the alternating directions of magnetic moments on individual atoms and the resulting zero net magnetization. However, relativistic quantum mechanics allows for generating current-induced internal fields whose sign alternates with the periodicity of the antiferromagnetic lattice. Using these fields, which couple strongly to the antiferromagnetic order, we demonstrate room-temperature electrical switching between stable configurations in antiferromagnetic CuMnAs thin-film devices by applied current with magnitudes of order 10(6) ampere per square centimeter. Electrical writing is combined in our solid-state memory with electrical readout and the stored magnetic state is insensitive to and produces no external magnetic field perturbations, which illustrates the unique merits of antiferromagnets for spintronics.
Manson, J. L.; Warter, M. L.; Schlueter, J. A.; Lancaster, T.; Steele, A. J.; Blundell, S. J.; Pratt, F. L.; Singleton, J.; McDonald, R. D.; Lee, C.; Whangbo, M.-H.; Plonczak, A. (Materials Science Division); (Eastern Washington Univ.); (Oxford Univ.); (Rutherford Appleton Lab.); (LANL); (North Carolina State Univ.)
2011-01-14
The two-dimensional antiferromagnet [Cu(HF{sub 2}){sub 2}(pyz)]{sub n} (pyz=pyrazine) has a rectangular lattice (see picture) displaying two types of FHF{sup -} bridging modes. The spin exchange through Cu-(FHF){sub 2}-Cu is about 90% stronger than through Cu-pyz-Cu, and the {mu}{sub 1,1}-coordinated FHF{sup -}, which is close in nature to F{sup -}---HF, is largely responsible for the exchange. C black, Cu red, F green, H cyan.
A spin-1 kagome antiferromagnet
Tovar, Mayra; Shtengel, Kirill; Refael, Gil
2010-03-01
We study a spin-1 antiferromagnet on the kagom'e lattice. We start by constructing a Klein-type SU(2) symmetric Hamiltonian which contains Heisenberg interactions between nearest and next-nearest neighbors as well as three-body terms. Our model Hamiltonian has an extensive degenerate ground state whose manifold is spanned by the AKLT-like valence bond states. We also perturb the parent Hamiltonian by introducing an enhancement to the nearest neighbor antiferromagnetic Heisenberg interactions. By projecting this perturbation onto the basis spanned by the unperturbed ground states, we derive an effective Hamiltonian which is dual to that of the transverse field antiferromagnetic Ising model on the triangular lattice. Based on the parameters of our model, we find it to be in the order-by-disorder phase. The ground state is a valence bond crystal stabilized by quantum fluctuations. We also discuss excitations, both magnetic and non-magnetic, and address their possible relevance to experiment.
Amaya, Naoki; Ono, Toshio; Oku, Yuta; Yamaguchi, Hironori; Matsuo, Akira; Kindo, Koichi; Nojiri, Hiroyuki; Palacio, Fernando; Campo, Javier; Hosokoshi, Yuko
2017-07-01
We have succeeded in synthesizing a new organic biradical F4BIPBNN [= 2,2'-(3,3',5,5'-tetrafluorobiphenyl-4,4'-diyl)bis(4,4,5,5-tetramethylimidazolin-1-oxyl 3-oxide)] which forms an S = 1/2 Heisenberg three-dimensional honeycomb antiferromagnet. Each site of a honeycomb layer alternately couples with upper or lower layers, which results in the unique three-dimensional honeycomb network with four nearest neighbors. At zero magnetic field, antiferromagnetic long-range order has been observed below TN = 2.7 K. Magnetic susceptibility in both paramagnetic and antiferromagnetic states and the magnetization curves are well reproduced by quantum Monte Carlo calculations with three antiferromagnetic interactions in the range of 4.3 to 6.6 K. From the concave shape of the magnetization curve, the shrinkage of spin due to spin fluctuations is evaluated to approximately 30% with respect to its classical value. The phase diagram of magnetic field versus temperature was determined by heat capacity and magnetization. In the field region below 3 T, a slight increase of TN was observed, which reflects the effect of spin fluctuations.
Jain, Avni; Errington, Jeffrey R; Truskett, Thomas M
2013-10-14
We use molecular simulation to construct equilibrium phase diagrams for two recently introduced model materials with isotropic, soft-repulsive pair interactions designed to favor diamond and simple cubic lattice ground states, respectively, over a wide range of densities [Jain et al., Soft Matter 9, 3866 (2013)]. We employ free energy based Monte Carlo simulation techniques to precisely trace the inter-crystal and fluid-crystal coexistence curves. We find that both model materials display rich polymorphic phase behavior featuring stable crystals corresponding to the target ground-state structures, as well as a variety of other crystalline (e.g., hexagonal and body-centered cubic) phases and multiple reentrant melting transitions.
Maasa Nakano
2013-04-01
Full Text Available Micrometer order magnetophotonic crystals with periodic arranged metallic glass and oxide glass composite materials were fabricated by stereolithographic method to reflect electromagnetic waves in terahertz frequency ranges through Bragg diffraction. In the fabrication process, the photo sensitive acrylic resin paste mixed with micrometer sized metallic glass of Fe72B14.4Si9.6Nb4 and oxide glass of B2O3·Bi2O3 particles was spread on a metal substrate, and cross sectional images of ultra violet ray were exposed. Through the layer by layer stacking, micro lattice structures with a diamond type periodic arrangement were successfully formed. The composite structures could be obtained through the dewaxing and sintering process with the lower temperature under the transition point of metallic glass. Transmission spectra of the terahertz waves through the magnetophotonic crystals were measured by using a terahertz time domain spectroscopy.
Katayama, Kazuya; Kurita, Nobuyuki; Tanaka, Hidekazu
2015-06-01
We have systematically investigated the variation of the exchange parameters and the ground state in the S =1/2 kagome-lattice antiferromagnet (Rb1 -xCsx )2Cu3SnF12 via magnetic measurements using single crystals. One of the parent compounds, Rb2Cu3SnF12 , which has a distorted kagome lattice accompanied by four sorts of nearest-neighbor exchange interaction, has a disordered ground state described by a pinwheel valence-bond-solid state. The other parent compound, Cs2Cu3SnF12 , which has a uniform kagome lattice at room temperature, has an ordered ground state with the q =0 spin structure. The analysis of magnetic susceptibilities shows that with increasing cesium concentration x , the exchange parameters increase with the tendency to be uniform. It was found that the ground state is disordered for x 0.53 . The pseudogap observed for x 0.53 approach zero at xc≃0.53 . This is indicative of the occurrence of a quantum phase transition at xc.
Li, Yanlu; Fan, Weiliu; Sun, Honggang; Cheng, Xiufeng; Li, Pan; Zhao, Xian
2011-06-01
Li2CdGeS4 and Li2CdSnS4 are novel quaternary diamond-like semiconductors (DLSs) which have been synthesized recently. We present first-principles calculations of their electronic, optical and lattice dynamic properties with the plane-wave pseudopotential method. We have found an indirect band gap of 2.78 eV for Li2CdGeS4 and a direct band gap of 2.50 eV for Li2CdSnS4. The serious stretching vibrations of the Ge/Sn-S and Li-S bonds may enhance their phonon energies, and cause them to exhibit high heat capacities and Debye temperatures, which are promising for nonlinear optical applications. Compared with Cu-based DLSs, Li plays a key role in enlarging the band gaps and increasing the lattice phonon energies, which would increase the thermal conductivity accompanied by an increase of the optical damage threshold.
Xu, Xun; Okada, Kunihide; Fujii, Muneaki [Department of Physics, Kumamoto University, Kurokami 2-39-1, Kumamoto 860 (Japan); Kubo, Takeji [Department of Physics, Nara Education University, Takabatake, Nara 613 (Japan); Ajiro, Yoshitami [Department of Applied Physics, Fukui University, Bunkyo 3-9-1, Fukui 910 (Japan)
1996-05-27
The Br NMR in the triangular-lattice antiferromagnetic CsMnBr{sub 3} is investigated in the ordered state at low temperatures. Two distinct peaks of the Br NMR spin-echo spectrum were observed at 36.0 {+-} 0.5 MHz and 43.0 {+-} 0.5 MHz accompanied by a broad signal ranging from 34 to 55 MHz in zero field. The peak frequencies are independent of temperature and the ratio of the frequencies is the same as that of the quadrupole moments of {sup 81}Br and {sup 79}Br. This suggests that the quadrupole resonance of Br is perturbed by the distribution of the internal magnetic field. Theoretical results obtained under the assumption that the Mn spins have disordered structure in the c-plane due to the frustration effect agree with the experimental data. (author)
Huang, Yi-Zhen; Xi, Bin; Chen, Xi; Li, Wei; Wang, Zheng-Chuan; Su, Gang
2016-06-01
The quantum phase transition, scaling behaviors, and thermodynamics in the spin-1/2 quantum Heisenberg model with antiferromagnetic coupling J>0 in the armchair direction and ferromagnetic interaction J^{'}Heisenberg O(3) universality. A zero magnetization plateau is observed in the dimerized phase, whose width decreases with increasing α. A phase diagram in the coupling ratio α-magnetic field h plane is obtained, where four phases, including dimerized, stripe, canted stripe, and polarized, are identified. It is also unveiled that the temperature dependence of the specific heat C(T) for different α's intersects precisely at one point, similar to that of liquid ^{3}He under different pressures and several magnetic compounds under various magnetic fields. The scaling behaviors of Q_{2}, ρ, and C(T) are carefully analyzed. The susceptibility is compared with the experimental data to give the magnetic parameters of both compounds.
Liu, Junjie; Goddard, Paul A; Singleton, John; Brambleby, Jamie; Foronda, Francesca; Möller, Johannes S; Kohama, Yoshimitsu; Ghannadzadeh, Saman; Ardavan, Arzhang; Blundell, Stephen J; Lancaster, Tom; Xiao, Fan; Williams, Robert C; Pratt, Francis L; Baker, Peter J; Wierschem, Keola; Lapidus, Saul H; Stone, Kevin H; Stephens, Peter W; Bendix, Jesper; Woods, Toby J; Carreiro, Kimberly E; Tran, Hope E; Villa, Cecelia J; Manson, Jamie L
2016-04-01
The crystal structures of NiX2(pyz)2 (X = Cl (1), Br (2), I (3), and NCS (4)) were determined by synchrotron X-ray powder diffraction. All four compounds consist of two-dimensional (2D) square arrays self-assembled from octahedral NiN4X2 units that are bridged by pyz ligands. The 2D layered motifs displayed by 1-4 are relevant to bifluoride-bridged [Ni(HF2)(pyz)2]EF6 (E = P, Sb), which also possess the same 2D layers. In contrast, terminal X ligands occupy axial positions in 1-4 and cause a staggered packing of adjacent layers. Long-range antiferromagnetic (AFM) order occurs below 1.5 (Cl), 1.9 (Br and NCS), and 2.5 K (I) as determined by heat capacity and muon-spin relaxation. The single-ion anisotropy and g factor of 2, 3, and 4 were measured by electron-spin resonance with no evidence for zero-field splitting (ZFS) being observed. The magnetism of 1-4 spans the spectrum from quasi-two-dimensional (2D) to three-dimensional (3D) antiferromagnetism. Nearly identical results and thermodynamic features were obtained for 2 and 4 as shown by pulsed-field magnetization, magnetic susceptibility, as well as their Néel temperatures. Magnetization curves for 2 and 4 calculated by quantum Monte Carlo simulation also show excellent agreement with the pulsed-field data. Compound 3 is characterized as a 3D AFM with the interlayer interaction (J⊥) being slightly stronger than the intralayer interaction along Ni-pyz-Ni segments (J(pyz)) within the two-dimensional [Ni(pyz)2](2+) square planes. Regardless of X, J(pyz) is similar for the four compounds and is roughly 1 K.
Goto, Masato; Ueda, Hiroaki; Michioka, Chishiro; Matsuo, Akira; Kindo, Koichi; Yoshimura, Kazuyoshi
2016-09-01
We have investigated the crystal structure and magnetic properties of three kagome lattice antiferromagnets, Rb2Na Ti3F12 , Cs2Na Ti3F12 , and Cs2K Ti3F12 , using single crystals. These compounds represent a S =1 /2 kagome system consisting of magnetic Ti3 + ions, which is expected to have negligibly small Dzyaloshinsky-Moriya interaction. The structural analyses revealed that each of the three compounds has a slightly distorted kagome lattice. The distortion of the kagome lattice becomes small as the ionic radii of constituent alkali metals increase. All three compounds have nearly the same Weiss temperature of -45 K, and the ground states are disordered and strongly depend on the distortion. The ground states of Rb2Na Ti3F12 , Cs2Na Ti3F12 , and Cs2K Ti3F12 are found to be a two-component state including approximately 1/3 nearly free spins, a gapless disordered state, and a gapped disordered state, respectively. Our experimental results suggest that the ground state of the ideal S =1 /2 Heisenberg kagome lattice antiferromagnet is gapped. In addition, the magnetization curves of Cs2Na Ti3F12 and Cs2K Ti3F12 show anomalies at approximately 1/3 of the full magnetic moment of Ti3 +, which are a notable observation of signs of the theoretically proposed 1/3 magnetization plateau in S =1 /2 kagome antiferromagnets.
Olson, D.W.
2001-01-01
An overview of the industrial diamond industry is provided. More than 90 percent of the industrial diamond consumed in the U.S. and the rest of the world is manufactured diamond. Ireland, Japan, Russia, and the U.S. produce 75 percent of the global industrial diamond output. In 2000, the U.S. was the largest market for industrial diamond. Industrial diamond applications, prices for industrial diamonds, imports and exports of industrial diamonds, the National Defense Stockpile of industrial diamonds, and the outlook for the industrial diamond market are discussed.
Pires, A. S. T.
2017-01-01
I present in details the SU(N) Schwinger boson formalism, also known as flavor wave theory, that has been used several times in the literature. I use the method to study the ferroquadrupolar phase of a quantum biquadratic Heisenberg model with spin S=1 on the triangular lattice with third-nearest-neighbor interactions. Results for the phase diagram at zero temperature and the static and dynamical quadrupolar structure factors are presented. In principle, the results could be applied to NiGa2S4.
Gong, Shou-Shu; Zhu, W.; Sheng, D. N.; Yang, Kun
2017-05-01
The exotic normal state of iron chalcogenide superconductor FeSe, which exhibits vanishing magnetic order and possesses an electronic nematic order, triggered extensive explorations of its magnetic ground state. To understand its novel properties, we study the ground state of a highly frustrated spin-1 system with bilinear-biquadratic interactions using an unbiased large-scale density matrix renormalization group. Remarkably, with increasing biquadratic interactions, we find a paramagnetic phase between Néel and stripe magnetic ordered phases. We identify this phase as a candidate of nematic quantum spin liquid by the compelling evidences, including vanished spin and quadrupolar orders, absence of lattice translational symmetry breaking, and a persistent nonzero lattice nematic order in the thermodynamic limit. The established quantum phase diagram naturally explains the observations of enhanced spin fluctuations of FeSe in neutron scattering measurement and the phase transition with increasing pressure. This identified paramagnetic phase provides a possibility to understand the novel properties of FeSe.
各向异性金刚石结构的光子晶体%Anisotropic Photonic Crystals with Diamond Lattice
詹仪; 郑义; 李效增; 李秀霞
2009-01-01
基于平面波展开法,理论分析了填充率、介质各向异性的程度对单轴金刚石结构三维光子晶体禁带的影响.结果表明,当填充率和介质各向异性取合适的值,单轴各向异性金刚石结构光子晶体存在着完全带隙.介质各向异性的引入使该晶体的带隙变窄甚至完全关闭.在各个布里渊区域里,带隙率和带隙宽度随介质各向异性程度的变化而变化.各向异性的引入为调整光子禁带提供了一种方法.%With the plane-wave expansion method, the photonic-band-gap structure for a diamond lattice consisting of a uniaxial anisotropic-dielectric sphere in air was studied through tuning three inequivalent 1/3 Brillouin zone. The results show that choosing the suitable range of filling fraction and anisotropy, a full band gap opens in the whole Brillouin zone for this anisotropic PBG structure. The gap to midgap ratio and bandgap width is tunable as a result of the changing extraordinary axis orientation of the uniaxial sphere. Anisotropy in sphere dielectric function is found to narrow or even close band gaps. The band gap width and close rate are affected by the extraordinary axis directions and anisotropy. The results in turn suggest a potential approach to obtain some degree of tunability of the photonic band structures.
Ghorbani, Elaheh; Shahbazi, Farhad; Mosadeq, Hamid
2016-10-12
Using the modified spin wave method, we study the [Formula: see text] Heisenberg model with first and second neighbor antiferromagnetic exchange interactions. For a symmetric S = 1/2 model, with the same couplings for all the equivalent neighbors, we find three phases in terms of the frustration parameter [Formula: see text]: (1) a commensurate collinear ordering with staggered magnetization (Néel.I state) for [Formula: see text], (2) a magnetically gapped disordered state for [Formula: see text], preserving all the symmetries of the Hamiltonian and lattice, which by definition is a quantum spin liquid (QSL) state and (3) a commensurate collinear ordering in which two out of the three nearest neighbor magnetizations are antiparallel and the remaining pair are parallel (Néel.II state), for [Formula: see text]. We also explore the phase diagram of a distorted [Formula: see text] model with S = 1/2. Distortion is introduced as an inequality of one nearest neighbor coupling with the other two. This yields a richer phase diagram by the appearance of a new gapped QSL, a gapless QSL and also a valence bond crystal phase in addition to the previous three phases found for the undistorted model.
Ghorbani, Elaheh; Shahbazi, Farhad; Mosadeq, Hamid
2016-10-01
Using the modified spin wave method, we study the {{J}1}-{{J}2} Heisenberg model with first and second neighbor antiferromagnetic exchange interactions. For a symmetric S = 1/2 model, with the same couplings for all the equivalent neighbors, we find three phases in terms of the frustration parameter \\barα={{J}2}/{{J}1} : (1) a commensurate collinear ordering with staggered magnetization (Néel.I state) for 0≤slant \\barα≲ 0.207 , (2) a magnetically gapped disordered state for 0.207≲ \\barα≲ 0.369 , preserving all the symmetries of the Hamiltonian and lattice, which by definition is a quantum spin liquid (QSL) state and (3) a commensurate collinear ordering in which two out of the three nearest neighbor magnetizations are antiparallel and the remaining pair are parallel (Néel.II state), for 0.396≲ \\barα≤slant 1 . We also explore the phase diagram of a distorted {{J}1}-{{J}2} model with S = 1/2. Distortion is introduced as an inequality of one nearest neighbor coupling with the other two. This yields a richer phase diagram by the appearance of a new gapped QSL, a gapless QSL and also a valence bond crystal phase in addition to the previous three phases found for the undistorted model.
Bhattacharjee, Suraka; Chaudhury, Ranjan
2016-11-01
The generalized spin stiffness constant for a doped quantum antiferromagnet has been investigated both analytically and numerically as a function of doping concentration at zero temperature, based on the strongly correlated t-J model on two-dimensional square lattice. The nature of the theoretical dependence of the stiffness constant on doping shows a striking similarity with that of the effective exchange constant, obtained from the combination of other theoretical and experimental techniques in the low doping region. This correspondence once again establishes that spin stiffness can very well play the role of an effective exchange constant even in the strongly correlated semi-itinerant systems. Our theoretical plot of the stiffness constant against doping concentration in the whole doping region exhibits the various characteristic features like a possible crossover in the higher doping regions and persistence of short range ordering even for very high doping with the complete vanishing of spin stiffness occurring only close to 100% doping. Our results receive very good support from various other theoretical approaches and also brings out a few limitations of some of them. Our detailed analysis highlights the crucial importance of the study of spin stiffness for the proper understanding of magnetic correlations in a semi-itinerant magnetic system described by the strongly correlated t-J model. Moreover, our basic formalism can also be utilized for determination of the effective exchange constant and magnetic correlations for itinerant magnetic systems, in general in a novel way.
Suh, B J
2000-01-01
A comprehensive analysis of the sup 3 sup 5 Cl nuclear magnetic resonance (NMR) relaxation data in Sr sub 2 CuO sub 2 Cl sub 2 single crystals is presented. Both the spin-lattice relaxation rate, T sub 1 sup - sup 1 (=2W), and the spin-spin relaxation rate, T sub 2 sup - sup 1 , show a crossover of the spin dimensionality well above the Neel temperature T sub N. The crossover is due to easy-plane anisotropy and is apparently signaled by the partial suppression of the Cu sup 2 sup + spin fluctuations along the tetragonal c-axis. By analyzing 2W for H ll c in terms of the critical behavior of the spin correlation length, we estimate the temperature for the crossover of the Cu sup 2 sup + spin correlations from Heisenberg to XY-like behavior to be T approx =290 K.
F Keshavarz
2017-02-01
Full Text Available In this study, the effect of four-spin exchanges between the nearest and next nearest neighbor spins of honeycomb lattice on the phase diagram of S=3/2 antiferomagnetic Heisenberg model is considered with two-spin exchanges between the nearest and next nearest neighbor spins. Firstly, the method is investigated with classical phase diagram. In classical phase diagram, in addition to Neel order, classical degeneracy is also seen. The existance of this phase in diagram phase is important because of the probability of the existence of quantum spin liquid in this region for such amount of interaction. To investigate the effect of quantum fluctuation on the stability of the obtained classical phase diagram, linear spin wave theory has been used. Obtained results show that in classical degeneracy regime, the quantum fluctuations cause the order by disorder in the spin system and the ground state is ordered
The electronic structure of antiferromagnetic chromium
Skriver, Hans Lomholt
1981-01-01
The author has used the local spin density formalism to perform self-consistent calculations of the electronic structure of chromium in the non-magnetic and commensurate antiferromagnetic phases, as a function of the lattice parameter. A change of a few per cent in the atomic radius brings...
Quantum Entanglement in Heisenberg Antiferromagnets
Subramanian, V
2004-01-01
Entanglement sharing among pairs of spins in Heisenberg antiferromagnets is investigated using the concurrence measure. For a nondegenerate S=0 ground state, a simple formula relates the concurrence to the diagonal correlation function. The concurrence length is seen to be extremely short. A few finite clusters are studied numerically, to see the trend in higher dimensions. It is argued that nearest-neighbour concurrence is zero for triangular and Kagome lattices. The concurrences in the maximal-spin states are explicitly calculated, where the concurrence averaged over all pairs is larger than the S=0 states.
Frustrated 3×3 Heisenberg antiferromagnets
Moustanis, P. N.
2016-08-01
The full energy spectrum and the exact thermodynamic results of the antiferromagnetic Heisenberg Hamiltonian of the 3×3 triangular and the frustrated square lattice with periodic boundary conditions and s=1/2 are obtained. To this end the method of hierarchy of algebras is employed. It was found that the ground state of the 3×3 frustrated square lattice is a Resonating Valence Bond (RVB) state. Thermodynamic properties, like the specific heat, magnetic susceptibility, the thermal average of the square of the total Sz and entropy, for these two lattices are presented.
Sera, A.; Kousaka, Y.; Akimitsu, J.; Sera, M.; Kawamata, T.; Koike, Y.; Inoue, K.
2016-12-01
We have performed the detailed investigations of the magnetization of the S =1/2 triangular-lattice antiferromagnets Ba3CoSb2O9 and CsCuCl3 with a 120∘ spin structure in the a b plane. In Ba3CoSb2O9 , the magnetic susceptibility (χ ) exhibits a broad maximum above the Néel temperature (TN) as is expected in the low-dimensional antiferromagnet (AFM). In CsCuCl3, χ exhibits a continuous increase down to TN as if it is the three-dimensional AFM. This is induced by the strong ferromagnetic (FM) interaction along the c axis. The magnetic phase diagrams are also very different. Although the transition field from the umbrella to the 2-1-coplanar phase (Hu -c) for H ∥c is almost independent of temperature in Ba3CoSb2O9 , it shows a considerable decrease with increasing temperature in CsCuCl3. The temperature independent Hu -c in Ba3CoSb2O9 originates from the magnetic anisotropy from the van Vleck contribution, which does not depend so much on the temperature. The temperature dependent Hu -c in CsCuCl3 originates from the magnetic anisotropy from the Dzyaloshinskii-Moriya (DM) interaction, which decreases with increasing temperature. For H ∥a b , the clear transition from the Y-coplanar to the up-up-down (u u d ) phase was observed in Ba3CoSb2O9 but not in CsCuCl3. While the reentrant behavior of TN originating from the thermal and quantum spin fluctuations is observed in both compounds, it is pronounced in Ba3CoSb2O9 but small in CsCuCl3. These differences originate from the existence or nonexistence of the DM interaction. The DM interaction in CsCuCl3 suppresses those fluctuations in the a b plane, leading to the less pronounced reentrant behavior of TN and the broad crossover in place of the phase transition. We analyzed the anisotropic magnetization of Ba3CoSb2O9 in the paramagnetic region by the mean field calculation. The spin-orbit (SO) coupling, the uniaxial crystalline electric field, and the isotropic exchange interaction were taken into account. We
Olson, D.W.
2013-01-01
Estimated 2012 world production of natural and synthetic industrial diamond was about 4.45 billion carats. During 2012, natural industrial diamonds were produced in at least 20 countries, and synthetic industrial diamond was produced in at least 12 countries. About 99 percent of the combined natural and synthetic global output was produced in Belarus, China, Ireland, Japan, Russia, South Africa and the United States. During 2012, China was the world’s leading producer of synthetic industrial diamond followed by the United States and Russia. In 2012, the two U.S. synthetic producers, one in Pennsylvania and the other in Ohio, had an estimated output of 103 million carats, valued at about $70.6 million. This was an estimated 43.7 million carats of synthetic diamond bort, grit, and dust and powder with a value of $14.5 million combined with an estimated 59.7 million carats of synthetic diamond stone with a value of $56.1 million. Also in 2012, nine U.S. firms manufactured polycrystalline diamond (PCD) from synthetic diamond grit and powder. The United States government does not collect or maintain data for either domestic PCD producers or domestic chemical vapor deposition (CVD) diamond producers for quantity or value of annual production. Current trade and consumption quantity data are not available for PCD or for CVD diamond. For these reasons, PCD and CVD diamond are not included in the industrial diamond quantitative data reported here.
Classical and quantum anisotropic Heisenberg antiferromagnets
W. Selke
2009-01-01
Full Text Available We study classical and quantum Heisenberg antiferromagnets with exchange anisotropy of XXZ-type and crystal field single-ion terms of quadratic and quartic form in a field. The magnets display a variety of phases, including the spin-flop (or, in the quantum case, spin-liquid and biconical (corresponding, in the quantum lattice gas description, to supersolid phases. Applying ground-state considerations, Monte Carlo and density matrix renormalization group methods, the impact of quantum effects and lattice dimension is analysed. Interesting critical and multicritical behaviour may occur at quantum and thermal phase transitions.
Spatially anisotropic Heisenberg kagome antiferromagnet
Apel, W.; Yavors'kii, T.; Everts, H.-U.
2007-04-01
In the search for spin-1/2 kagome antiferromagnets, the mineral volborthite has recently been the subject of experimental studies (Hiroi et al 2001 J. Phys. Soc. Japan 70 3377; Fukaya et al 2003 Phys. Rev. Lett. 91 207603; Bert et al 2004 J. Phys.: Condens. Matter 16 S829; Bert et al 2005 Phys. Rev. Lett. 95 087203). It has been suggested that the magnetic properties of this material are described by a spin-1/2 Heisenberg model on the kagome lattice with spatially anisotropic exchange couplings. We report on investigations of the {\\mathrm {Sp}}(\\mathcal {N}) symmetric generalization of this model in the large \\mathcal {N} limit. We obtain a detailed description of the dependence of possible ground states on the anisotropy and on the spin length S. A fairly rich phase diagram with a ferrimagnetic phase, incommensurate phases with and without long-range order and a decoupled chain phase emerges.
Antiferromagnetic Ising Model in Hierarchical Networks
Cheng, Xiang; Boettcher, Stefan
2015-03-01
The Ising antiferromagnet is a convenient model of glassy dynamics. It can introduce geometric frustrations and may give rise to a spin glass phase and glassy relaxation at low temperatures [ 1 ] . We apply the antiferromagnetic Ising model to 3 hierarchical networks which share features of both small world networks and regular lattices. Their recursive and fixed structures make them suitable for exact renormalization group analysis as well as numerical simulations. We first explore the dynamical behaviors using simulated annealing and discover an extremely slow relaxation at low temperatures. Then we employ the Wang-Landau algorithm to investigate the energy landscape and the corresponding equilibrium behaviors for different system sizes. Besides the Monte Carlo methods, renormalization group [ 2 ] is used to study the equilibrium properties in the thermodynamic limit and to compare with the results from simulated annealing and Wang-Landau sampling. Supported through NSF Grant DMR-1207431.
Antiferromagnetic order in hybrid electromagnetic metamaterials
Miroshnichenko, Andrey E.; Filonov, Dmitry; Lukyanchuk, Boris; Kivshar, Yuri
2017-08-01
We demonstrate experimentally a new type of order in optical magnetism resembling the staggered structure of spins in antiferromagnetic ordered materials. We study hybrid electromagnetic metasurfaces created by assembling hybrid meta-atoms formed by metallic split-ring resonators and dielectric particles with a high refractive index, both supporting optically-induced magnetic dipole resonances of different origin. Each pair (or ‘metamolecule’) is characterized by two interacting magnetic dipole moments with the distance-dependent magnetization resembling the spin exchange interaction in magnetic materials. By directly mapping the structure of the electromagnetic fields, we demonstrate experimentally that strong coupling between the optically-induced magnetic moments of different origin can flip the magnetisation orientation in a metamolecule creating an antiferromagnetic lattice of staggered optically-induced magnetic moments in hybrid metasurfaces.
Antiferromagnetic exchange mechanism of superconductivity in cuprates
Plakida, N M
2001-01-01
One examines theory of superconducting coupling resulted from antiferromagnetic exchange in terms of which one explains strong dependence of T sub c superconducting transition temperature on alpha lattice constant. Calculations are based on the Hubbard p-d two-region model within strong correlation limit. DELTA pd excitation high energy at antiferromagnetic exchange of two particles from different Hubbard subregions results in suppression o delay effects and in coupling of all particles in conductivity subregion with Fermi energy E sub F >= DELTA pd : T sub c approx = E sub F exp(-1/lambda), where lambda propor to J. T sub c (alpha) and isotopic effect are explained by J exchange interaction dependence on alpha and on zero oscillations of oxygen ions
Singleton, John [Los Alamos National Laboratory; Mc Donald, R [Los Alamos National Laboratory; Sengupta, P [Los Alamos National Laboratory; Cox, S [Los Alamos National Laboratory; Manson, J [E WASHINGTON U; Southerland, H [E WASHINGTON U; Warter, M [E WASHINGTON U; Stone, K [STATE UNIV OF NY; Stephens, P [STATE UNIV OF NY; Lancaster, T [OXFORD U; Steele, A [OXFORD U; Blundell, S [OXFORD U; Baker, P [OXFORD U; Pratt, F [RUTHERFORD-APPLETON LAB; Lee, C [NCSU; Whangbo, M [NCSU
2009-01-01
X-ray powder diffraction and magnetic susceptibility measurements show that Ag(pyz){sub 2}(S{sub 2}O{sub 8}) consists of 2D square nets of Ag{sup 2+} ions resulting from the corner-sharing of axially elongated AgN{sub 4}O{sub 2} octahedra and exhibits characteristic 2D antiferromagnetism. Nevertheless, {mu}{sup +}Sr measurements indicate that Ag(pyz){sub 2}(S{sub 2}O{sub 8}) undergoes 3D magnetic ordering below 7.8(3) K.
Aharonovich, Igor
2014-01-01
The burgeoning field of nanophotonics has grown to be a major research area, primarily because of the ability to control and manipulate single quantum systems (emitters) and single photons on demand. For many years studying nanophotonic phenomena was limited to traditional semiconductors (including silicon and GaAs) and experiments were carried out predominantly at cryogenic temperatures. In the last decade, however, diamond has emerged as a new contender to study photonic phenomena at the nanoscale. Offering plethora of quantum emitters that are optically active at room temperature and ambient conditions, diamond has been exploited to demonstrate super-resolution microscopy and realize entanglement, Purcell enhancement and other quantum and classical nanophotonic effects. Elucidating the importance of diamond as a material, this review will highlight the recent achievements in the field of diamond nanophotonics, and convey a roadmap for future experiments and technological advancements.
Electronic structures of phosphorus-doped diamond films and impacts of their vacancies
无
2010-01-01
In order to better understand the bonding mechanisms of the phosphorus-doped diamond films and the influences of the phosphorus-doped concentration on the diamond lattice integrity and conductivity,we calculate the electronic structures of the phosphorus-doped diamond with different phosphorus concentrations and the density of states in the phosphorus--doped diamond films with a vacant lattice site by the first principle method.The calculation results show the phosphorus atom only affects the bonds of a few atoms in its vicinity,and the conductivity increases as the doped concentration increases.Also in the diamond lattice with a total number of 64 atoms and introducing a vacancy into the non-nearest neighbor lattice site of a phosphorus atom,we have found that both the injuries of the phosphorus-doped diamond films and the N-type electron conductivity of diamond films could be improved.
Antiferromagnetic spin-orbitronics
Manchon, Aurelien
2015-05-01
Antiferromagnets have long remained an intriguing and exotic state of matter, whose application has been restricted to enabling interfacial exchange bias in metallic and tunneling spin-valves [1]. Their role in the expanding field of applied spintronics has been mostly passive and the in-depth investigation of their basic properties mostly considered from a fundamental perspective.
Nanoparticles of antiferromagnetic materials
Madsen, Daniel Esmarch
2008-01-01
I denne Ph.D. afhandling studeres forskellige egenskaber ved antiferromagnetiske nanopartikler. I en ideel antiferromagnet er spinnene orienteret således at der ikke er et resulterende magnetisk moment. I nanopartikler af antiferromagnetiske materialer er denne kompensation på grund af forskellig...
High-pressure-high-temperature treatment of natural diamonds
Royen, J V
2002-01-01
The results are reported of high-pressure-high-temperature (HPHT) treatment experiments on natural diamonds of different origins and with different impurity contents. The diamonds are annealed in a temperature range up to 2000 sup o C at stabilizing pressures up to 7 GPa. The evolution is studied of different defects in the diamond crystal lattice. The influence of substitutional nitrogen atoms, plastic deformation and the combination of these is discussed. Diamonds are characterized at room and liquid nitrogen temperature using UV-visible spectrophotometry, Fourier transform infrared spectrophotometry and photoluminescence spectrometry. The economic implications of diamond HPHT treatments are discussed.
Barlowite: A Spin-1/2 Antiferromagnet with a Geometrically Perfect Kagome Motif.
Han, Tian-Heng; Singleton, John; Schlueter, John A
2014-11-28
We present thermodynamic studies of a new spin-1/2 antiferromagnet containing undistorted kagome lattices-barlowite Cu_{4}(OH)_{6}FBr. Magnetic susceptibility gives θ_{CW}=-136 K, while long-range order does not happen until T_{N}=15 K with a weak ferromagnetic moment μkagome lattice makes charge doping promising.
Holes in Heisenberg antiferromagnets
Chen, Yang
1990-05-01
In this Brief Report we show that a recent model proposed by Shankar [Phys. Rev. Lett. 63, 203 (1989)], describing the motion of holes in quantum antiferromagnets is equivalent to the Schwinger model [Phys. Rev. 128, 2425 (1962)] in 1+1 dimensions. Some exact results are deduced. In addition to the superconducting long-range order found by Shankar, it is shown that there is a 2pF hole density wave existing with the superconducting pairing instability.
Analysis of the carbon source for diamond crystal growth
LI Li; XU Bin; LI MuSen
2008-01-01
The lattice constants of diamond and graphite at high pressure and high temperature (HPHT) were calculated on the basis of linear expansion coefficient and elastic constant. According to the empirical electron theory of solids and molecules (EET), the valence electron structures (VESs) of diamond, graphite crystal and their common planes were calculated. The relationship between diamond and graphite structure was analyzed based on the boundary condition of the improved Thomas-Fermi-Dirac theory by Cheng (TFDC). It was found that the electron densities of common planes in graphite were not continuous with those of planes in diamond at the first order of approximation. The results show that during the course of diamond single crystal growth at HPHT with metal catalyst, the carbon sources forming diamond structure do not come from the graphite structure directly. The diamond growth mechanism was discussed from the viewpoint of valence electron structure.
Magnetic and structural properties of antiferromagnetic VF{sub 3}
Reuvekamp, Patrick; Kremer, Reinhard; Eger, Roland [Max-Planck-Institut fuer Festkoerperforschung, Heisenbergstrasse 1, D-70569 Stuttgart (Germany); Nenert, Gwilherm; Hansen, Thomas [Institut Laue-Langevin, 38042 Grenoble (France)
2013-07-01
We report on a magnetic and structural investigation of layered antiferromagnetic system vanadium (III) fluoride. VF{sub 3} crystallizes in a distorted ReO{sub 3} structure (R anti 3c) with rotated undistorted VF{sub 6} octahedra. The V{sup +3} cations are arranged in a triangular lattice with the possibility of exhibiting magnetic frustration. Polycrystalline samples of VF{sub 3} were investigated using heat capacity, dielectric, magnetic susceptibility and neutron powder diffraction methods. Combining our results, we confirmed that VF{sub 3} undergoes long-range antiferromagnetic order at ∝19 K in accordance with literature. The antiferromagnetic order results in a magnetic structure with the magnetic moments alternating between a parallel and b parallel alignments in the ab plane. A second phase transition can be seen at ∝120 K in the heat capacity and dielectric measurements possibly associated to a minute structural distortion.
Magnetic phase diagrams of classical triangular and kagome antiferromagnets
Gvozdikova, M V [Department of Physics, Kharkov National University, 61077 Kharkov (Ukraine); Melchy, P-E; Zhitomirsky, M E, E-mail: mike.zhitomirsky@cea.fr [Service de Physique Statistique, Magnetisme et Supraconductivite, UMR-E9001 CEA-INAC/UJF, 17 rue des Martyrs, 38054 Grenoble (France)
2011-04-27
We investigate the effect of geometrical frustration on the H-T phase diagrams of the classical Heisenberg antiferromagnets on triangular and kagome lattices. The phase diagrams for the two models are obtained from large-scale Monte Carlo simulations. For the kagome antiferromagnet, thermal fluctuations are unable to lift degeneracy completely and stabilize translationally disordered multipolar phases. We find a substantial difference in the temperature scales of the order by disorder effect related to different degeneracy of the low- and the high-field classical ground states in the kagome antiferromagnet. In the low-field regime, the Kosterlitz-Thouless transition into a spin-nematic phase is produced by unbinding of half-quantum vortices.
Kondo Screening and Fermi Surface in the Antiferromagnetic Metal Phase
Yamamoto, Seiji; Si, Qimiao
2006-03-01
We address the Kondo effect deep inside the antiferromagnetic metal phase of a Kondo lattice Hamiltonian with SU(2) invariance. The local- moment component is described in terms of a non-linear sigma model. The Fermi surface of the conduction electron component is taken to be sufficiently small, so that it is not spanned by the antiferromagnetic wavevector. The effective low energy form of the Kondo coupling simplifies drastically, corresponding to the uniform component of the magnetization that forward-scatters the conduction electrons on their own Fermi surface. We use a combined bosonic and fermionic (Shankar) renormalization group procedure to analyze this effective theory and study the Kondo screening and Fermi surface in the antiferromagnetic phase. The implications for the global magnetic phase diagram, as well as quantum critical points, of heavy fermion metals are discussed.
Magnetic phase diagrams of classical triangular and kagome antiferromagnets.
Gvozdikova, M V; Melchy, P-E; Zhitomirsky, M E
2011-04-27
We investigate the effect of geometrical frustration on the H-T phase diagrams of the classical Heisenberg antiferromagnets on triangular and kagome lattices. The phase diagrams for the two models are obtained from large-scale Monte Carlo simulations. For the kagome antiferromagnet, thermal fluctuations are unable to lift degeneracy completely and stabilize translationally disordered multipolar phases. We find a substantial difference in the temperature scales of the order by disorder effect related to different degeneracy of the low- and the high-field classical ground states in the kagome antiferromagnet. In the low-field regime, the Kosterlitz-Thouless transition into a spin-nematic phase is produced by unbinding of half-quantum vortices.
Role of the antiferromagnetic bulk spins in exchange bias
Schuller, Ivan K. [Center for Advanced Nanoscience and Physics Department, University of California San Diego, La Jolla, CA 92093 (United States); Morales, Rafael, E-mail: rafael.morales@ehu.es [Department of Chemical-Physics & BCMaterials, University of the Basque Country UPV/EHU (Spain); IKERBASQUE, Basque Foundation for Science, 48011 Bilbao (Spain); Batlle, Xavier [Departament Física Fonamental and Institut de Nanociència i Nanotecnologia, Universitat de Barcelona, c/ Martí i Franqués s/n, 08028 Barcelona, Catalonia (Spain); Nowak, Ulrich [Department of Physics, University of Konstanz, 78464 Konstanz (Germany); Güntherodt, Gernot [Physics Institute (IIA), RWTH Aachen University, Campus RWTH-Melaten, 52074 Aachen (Germany)
2016-10-15
This “Critical Focused Issue” presents a brief review of experiments and models which describe the origin of exchange bias in epitaxial or textured ferromagnetic/antiferromagnetic bilayers. Evidence is presented which clearly indicates that inner, uncompensated, pinned moments in the bulk of the antiferromagnet (AFM) play a very important role in setting the magnitude of the exchange bias. A critical evaluation of the extensive literature in the field indicates that it is useful to think of this bulk, pinned uncompensated moments as a new type of a ferromagnet which has a low total moment, an ordering temperature given by the AFM Néel temperature, with parallel aligned moments randomly distributed on the regular AFM lattice. - Highlights: • We address the role of bulk antiferromagnetic spins in the exchange bias phenomenon. • Significant experiments on how bulk AFM spins determine exchange bias are highlighted. • We explain the model that accounts for experimental results.
Antiferromagnetic hedgehogs with superconducting cores
Goldbart, P.M.; Sheehy, D.E. [Department of Physics and Materials Research Laboratory, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801 (United States)
1998-09-01
Excitations of the antiferromagnetic state that resemble antiferromagnetic hedgehogs at large distances but are predominantly superconducting inside a core region are discussed within the context of Zhang{close_quote}s SO(5)-symmetry-based approach to the physics of high-temperature superconducting materials. Nonsingular, in contrast with their hedgehog cousins in pure antiferromagnetism, these texture excitations are what hedgehogs become when the antiferromagnetic order parameter is permitted to {open_quotes}escape{close_quotes} into superconducting directions. The structure of such excitations is determined in a simple setting, and a number of their experimental implications are examined. {copyright} {ital 1998} {ital The American Physical Society}
Artifact Diamond Its Allure And Significance
Yoder, Max N.
1989-01-01
While the preponderance of the mechanical, optical, and electronic properties of natural diamond have been known for over a decade, only recently has artifact diamond in technologically useful form factors become an exciting possibility. The advent of sacrificial, lattice matched crystalline substrates provides the basis not only for semiconducting applications of diamond, but for optical mirrors, lenses, and windows as well. As a semiconductor, diamond has the highest resistivity, the highest saturated electron velocity, the highest thermal conductivity, the lowest dielectric constant, the highest dielectric strength, the greatest hardness, the largest bandgap and the smallest lattice constant of any material. It also has electron and hole mobilities greater than those of silicon. Its figure of merit as a microwave power amplifier is unexcelled and exceeds that of silicon by a multiplier of 8200. For integrated circuit potential, its thermal conductivity, saturated velocity, and dielectric constant also place it in the premier position (32 times that of silicon, 46 times that of GaAs). Although not verified, its radiation hardness should also be unmatched. Aside from its brilliant sparkle as a gemstone, there has been little use of diamond in the field of optics. Processing of the diamond surface now appears to be as simple as that of any other material --albeit with different techniques. In fact, it may be possible to etch diamond far more controllably (at economically viable rates) than any other material as the product of the etch is gaseous and the etched trough is self-cleaning. Other properties of diamond make it an ideal optical material. Among them are its unmatched thermal conductivity, its extremely low absorption loss above 228 nanometers, and unmatched Young's modulus, Poisson's ratio, tensile strength, hardness, thermal shock, and modulus of elasticity. If the recently-found mechanisms by which erbium impurities in III-V junctions can be made to "lase
Jiang Qing; Zhong Chonggui
2002-12-30
Soft-mode theory based on DIFFOUR model for ferroelectric interaction and the mean-field theory of high spin Ising model for antiferromagnetic interaction are used to investigate the ferroelectric, antiferromagnetic, magnetoelectric properties in ferroelectromagnetic lattice in which the ferroelectric order and antiferromagnetic order coexist simultaneously below a certain temperature. Ferroelectric polarization, spin moment, and magnetoelectric susceptibility as well, as a function of temperature for system, are calculated and compared with the different coupling coefficient. It is found that an anomaly appears in curve of the polarization susceptibility as a function of temperature due to the coupling between the ferroelectric and antiferromagnetic orders in the ferroelectromagnetic lattice. At the same time, we also considered the influence of magnetoelectric effect on polarization susceptibility by applying the external field including electric and magnetic.
Antiferromagnetic spin Seebeck effect.
Wu, Stephen M.; Zhang, Wei; KC, Amit; Borisov, Pavel; Pearson, John E.; Jiang, J. Samuel; Lederman, David; Hoffmann, Axel; Bhattacharya, Anand
2016-03-03
We report on the observation of the spin Seebeck effect in antiferromagnetic MnF2. A device scale on-chip heater is deposited on a bilayer of MnF2 (110) (30nm)/Pt (4 nm) grown by molecular beam epitaxy on a MgF2(110) substrate. Using Pt as a spin detector layer, it is possible to measure the thermally generated spin current from MnF2 through the inverse spin Hall effect. The low temperature (2–80 K) and high magnetic field (up to 140 kOe) regime is explored. A clear spin-flop transition corresponding to the sudden rotation of antiferromagnetic spins out of the easy axis is observed in the spin Seebeck signal when large magnetic fields (>9T) are applied parallel to the easy axis of the MnF2 thin film. When the magnetic field is applied perpendicular to the easy axis, the spin-flop transition is absent, as expected.
Antiferromagnetic Spin Seebeck Effect
Wu, Stephen M.; Zhang, Wei; KC, Amit; Borisov, Pavel; Pearson, John E.; Jiang, J. Samuel; Lederman, David; Hoffmann, Axel; Bhattacharya, Anand
2016-03-01
We report on the observation of the spin Seebeck effect in antiferromagnetic MnF2 . A device scale on-chip heater is deposited on a bilayer of MnF2 (110) (30 nm )/Pt (4 nm) grown by molecular beam epitaxy on a MgF2 (110) substrate. Using Pt as a spin detector layer, it is possible to measure the thermally generated spin current from MnF2 through the inverse spin Hall effect. The low temperature (2-80 K) and high magnetic field (up to 140 kOe) regime is explored. A clear spin-flop transition corresponding to the sudden rotation of antiferromagnetic spins out of the easy axis is observed in the spin Seebeck signal when large magnetic fields (>9 T ) are applied parallel to the easy axis of the MnF2 thin film. When the magnetic field is applied perpendicular to the easy axis, the spin-flop transition is absent, as expected.
Spatially frustrated S = 1 Heisenberg antiferromagnet with single ion anisotropy
Pires, A. S. T.
2016-10-01
Using the SU(3) Schwinger boson formalism, I study the S = 1 square lattice Heisenberg antiferromagnet, at zero temperature, with spatially anisotropic nearest-neighbor couplings frustrated by a next-nearest neighbor interaction and single ion anisotropy. The phase diagram at zero temperature is presented. My calculations show two magnetically ordered phases separated by a quantum-disordered region for all values of the anisotropy.
Hida, Kazuo; Takano, Ken'ichi; Suzuki, Hidenori
2010-11-01
The ground states of two types of distorted mixed diamond chains with spins 1 and 1/2 are investigated using exact diagonalization, DMRG, and mapping onto low-energy effective models. In the undistorted case, the ground state consists of an array of independent spin-1 clusters separated by singlet dimers. The lattice distortion induces an effective interaction between cluster spins. When this effective interaction is antiferromagnetic, several Haldane phases appear with or without spontaneous translational symmetry breakdown (STSB). The transition between the Haldane phase without STSB and that with (n+1)-fold STSB (n=1, 2, and 3) belongs to the same universality class as the (n+1)-clock model. In contrast, when the effective interaction is ferromagnetic, the quantized and partial ferrimagnetic phases appear with or without STSB. An effective low-energy theory for the partial ferrimagnetic phase is presented.
Antiferromagnetic spin Seebeck Effect
Wu, SM; W. Zhang; Kc, A; Borisov, P.; Pearson, JE; Jiang, JS; Lederman, D.; Hoffmann, A.; Bhattacharya, A
2015-01-01
We report on the observation of the spin Seebeck effect in antiferromagnetic MnF_{2}. A device scale on-chip heater is deposited on a bilayer of MnF_{2} (110) (30 nm)/Pt (4 nm) grown by molecular beam epitaxy on a MgF_{2} (110) substrate. Using Pt as a spin detector layer, it is possible to measure the thermally generated spin current from MnF_{2} through the inverse spin Hall effect. The low temperature (2-80 K) and high magnetic field (up to 140 kOe) regime is explored. A clear spin-flop t...
Topological gapless phases in nonsymmorphic antiferromagnets
Brzezicki, Wojciech; Cuoco, Mario
2017-04-01
We investigate the nature of the electronic states in a variety of nonsymmorphic collinear antiferromagnets with glide reflection symmetry, a combination of mirror and half-lattice translation. In particular, the study refers to a class of systems with two-band itinerant electrons that are spin-orbit coupled and interacting with a magnetic background having a zigzag pattern. We describe the symmetry properties of the model system by focusing on the role of nonsymmorphic transformations arising from the antiferromagnetic structure of the spin ordering. Gapless phases with Dirac points having different types of symmetry-protection as well as electronic structures with triple and quadruple band-crossing points are obtained. A glide semimetal is shown to be converted into a gapless phase with Dirac points protected by inversion and time-inversion symmetry combination. Interestingly, we find a relation between the states in the glide sectors that provides a general mechanism to get multiple band touching points. The split of the multiple Fermi points drives the transition from a point node to a line node semimetal or to a metal with nontrivial winding around the Fermi pockets and an electronic structure that is tied to the presence of glide symmetric Dirac points. Besides a new perspective of ordered states in complex materials, our findings indicate relevant paths to topological gapless phases and edge states in a wide class of magnetic systems.
Landau model for the multiferroic delafossite antiferromagnets
Ribeiro, J. L.; Perez-Mato, J. M.; Vieira, L. G.
2016-10-01
A symmetry based framework is used to describe the complex phase diagrams observed in the multiferroic delafossite compounds. A free energy Landau functional is derived from the analysis of the transformation properties of the most general incommensurate magnetic spin order parameter. A principle of maximal symmetry is invoked and the stability of each of the different higher symmetry phases considered. The competition between different potential ground states is analysed within the scope of a simplified model, which emphasizes the role of the symmetry allowed phase dependent biquadratic couplings. The cross-over between the different competing states is also discussed. The results show that the diverse set of phase diagrams that are experimentally observed in this class of triangular lattice antiferromagnets and, in particular, the stabilization of magnetically induced ferroelectric states, can be well interpreted and described within this integrated phenomenological approximation.
Transformation of spin current by antiferromagnetic insulators
Khymyn, Roman; Lisenkov, Ivan; Tiberkevich, Vasil S.; Slavin, Andrei N.; Ivanov, Boris A.
2016-06-01
It is demonstrated theoretically that a thin layer of an anisotropic antiferromagnetic (AFM) insulator can effectively conduct spin current through the excitation of a pair of evanescent AFM spin wave modes. The spin current flowing through the AFM is not conserved due to the interaction between the excited AFM modes and the AFM lattice and, depending on the excitation conditions, can be either attenuated or enhanced. When the phase difference between the excited evanescent modes is close to π /2 , there is an optimum AFM thickness for which the output spin current reaches a maximum, which can significantly exceed the magnitude of the input spin current. The spin current transfer through the AFM depends on the ambient temperature and increases substantially when temperature approaches the Néel temperature of the AFM layer.
Probing the evolution of antiferromagnetism in multiferroics
Holcomb, M.; Martin, L.; Scholl, A.; He, Q.; Yu, P.; Yang, C.-H.; Yang, S.; Glans, P.-A.; Valvidares, M.; Huijben, M.; Kortright, J.; Guo,, J.; Chu, Y.-H.; Ramesh, R.
2010-06-09
This study delineates the evolution of magnetic order in epitaxial films of the room-temperature multiferroic BiFeO3 system. Using angle- and temperature-dependent dichroic measurements and spectromicroscopy, we have observed that the antiferromagnetic order in the model multiferroic BiFeO3 evolves systematically as a function of thickness and strain. Lattice-mismatch-induced strain is found to break the easy-plane magnetic symmetry of the bulk and leads to an easy axis of magnetization which can be controlled through strain. Understanding the evolution of magnetic structure and how to manipulate the magnetism in this model multiferroic has significant implications for utilization of such magnetoelectric materials in future applications.
von Reppert, A; Pudell, J; Koc, A; Reinhardt, M; Leitenberger, W; Dumesnil, K; Zamponi, F; Bargheer, M
2016-09-01
We present a temperature and fluence dependent Ultrafast X-Ray Diffraction study of a laser-heated antiferromagnetic dysprosium thin film. The loss of antiferromagnetic order is evidenced by a pronounced lattice contraction. We devise a method to determine the energy flow between the phonon and spin system from calibrated Bragg peak positions in thermal equilibrium. Reestablishing the magnetic order is much slower than the cooling of the lattice, especially around the Néel temperature. Despite the pronounced magnetostriction, the transfer of energy from the spin system to the phonons in Dy is slow after the spin-order is lost.
A. von Reppert
2016-09-01
Full Text Available We present a temperature and fluence dependent Ultrafast X-Ray Diffraction study of a laser-heated antiferromagnetic dysprosium thin film. The loss of antiferromagnetic order is evidenced by a pronounced lattice contraction. We devise a method to determine the energy flow between the phonon and spin system from calibrated Bragg peak positions in thermal equilibrium. Reestablishing the magnetic order is much slower than the cooling of the lattice, especially around the Néel temperature. Despite the pronounced magnetostriction, the transfer of energy from the spin system to the phonons in Dy is slow after the spin-order is lost.
Localized vibrational modes in diamond
Murzaev, R. T.; Bachurin, D. V.; Korznikova, E. A.; Dmitriev, S. V.
2017-03-01
Discrete breather (DB) or, synonymously, intrinsic localized mode (ILM) is a spatially localized and time-periodic vibrational mode in a defect-free nonlinear lattice, e.g., in a crystal lattice. Standing DB and DB clusters (double and triple) are studied in diamond using molecular dynamics method with the AIREBO interatomic potentials. Single DB can be easily excited by applying initial shifts, A0, to a pair of nearest atoms along the valence bond in the opposite directions. Admissible excitation amplitudes are 0.09 ≤A0 /a0 ≤ 0.12, where a0 is the equilibrium interatomic distance. The core of a DB is a pair of nearest carbon atoms oscillating out-of-phase, while the neighboring atoms oscillate with one order of magnitude lower amplitudes. DB frequency is above the top of the phonon spectrum and increases with the oscillation amplitude. DB lives for more than 100 oscillation periods which approximately corresponds to 2 ps. The range of initial amplitudes and other conditions necessary for the excitation of double and triple DB clusters as well as their lifetime are investigated in detail. Two different mechanisms of energy exchange between DBs in the DB clusters are revealed, which is the main result of the present study. Our results contribute to a deeper understanding of the nonlinear lattice dynamics of diamond.
Superconductivity, antiferromagnetism, and neutron scattering
Tranquada, John M., E-mail: jtran@bnl.gov; Xu, Guangyong; Zaliznyak, Igor A.
2014-01-15
High-temperature superconductivity in both the copper-oxide and the iron–pnictide/chalcogenide systems occurs in close proximity to antiferromagnetically ordered states. Neutron scattering has been an essential technique for characterizing the spin correlations in the antiferromagnetic phases and for demonstrating how the spin fluctuations persist in the superconductors. While the nature of the spin correlations in the superconductors remains controversial, the neutron scattering measurements of magnetic excitations over broad ranges of energy and momentum transfers provide important constraints on the theoretical options. We present an overview of the neutron scattering work on high-temperature superconductors and discuss some of the outstanding issues. - Highlights: • High-temperature superconductivity is closely associated with antiferromagnetism. • Antiferromagnetic spin fluctuations coexist with the superconductivity. • Neutron scattering is essential for characterising the full spectrum of spin excitations.
Hydrocarbons Encapsulated in Diamonds From China and India
Leung, I.; Tsao, C.; Taj-Eddin, I.
2005-05-01
We examined a large number of diamonds from a kimberlite pipe located in Fuxian, China, and alluvial diamonds from Panna, India. We selected 6-10 diamonds from each locality based on certain characteristics: they are white, brilliant, mostly devoid of mineral inclusions, fracture-free, many contain microscopic bubbles, some display etched circular patterns. These diamonds were examined under ultraviolet (UV) light using a fluorescence microscope, then, investigated using a Nicolet 6700 FT-IR spectrometer. Several diamonds emit blue fluorescence when excited with UV light, while others appear dim because they are not fluorescent. It is the latter that render the included bubbles clearly visible, glowing as yellow and blue spherules within the dim diamond host. These fluorescent bubbles are probably filled with hydrocarbon fluids of variable compositions. FT-IR spectra of diamond typically show absorption due to intrinsic diamond lattice vibrations. We found in most of our diamonds used in this study an additional, outstanding group of absorption bands located just below the wavenumber 3000. Peak positions in this region correlate well with symmetric and asymmetric stretching of methylene and methyl groups, attributable to H bonded to C atoms. Comparing them with standard spectral shapes, we found a good match with an alkane molecule composed of saturated aliphatic hydrocarbons. Our observations provide evidence that hydrocarbons might be important components in the deep mantle, but, to transport them up to Earth's surface would require strong capsules which, perhaps, only diamond could provide.
Inclusions of Hydrocarbon Fluids in Diamonds From Wafangdian, Liaoning, China
Leung, I. S.; Tsao, C.
2015-12-01
We studied a large number of industrial-grade diamonds from Pipe 50 of Liaoning, China. These diamonds are not suitable for polishing into gems or making cutting tools. They are usually crushed to form abrasives, without much scientific scrutiny. We report here fluid inclusions in dozens of diamonds. The first type of fluids occur in the outer rim of diamonds, just below the surface, while their interior is free of visible fluids. Under UV radiation, when a non-fluorescent diamond appeared dim, bubbles of included fluids became visible as yellow and blue spherules. Such diamonds are sometimes encrusted with euhedral micro-diamonds resembling those on thin films grown by CVD. The second type of fluid-rich diamonds display iridescence of pink, blue, green and yellow colors. They show lamellar, filamentous, or tubular structures, some of the tubes are filled with granules, probably grown from fluids in the tubes. An FT-IR investigation of both types yielded similar results. Apart from absorption due to intrinsic diamond lattice vibrations, we found an outstanding group of bands just below wavenumber 3000. This indicates the presence of a saturated aliphatic hydrocarbons of long chain length. Our results seem to implicate that hydrocarbons might be an important component in Earth's mantle, which might even have provided carbon from which diamonds crystllized.
Lattice effects in YVO3 single crystal
Marquina, C; Sikora, M; Ibarra, MR; Nugroho, AA; Palstra, TTM
2005-01-01
In this paper we report on the lattice effects in the Mott insulator yttrium orthovanadate (YVO3). Linear thermal expansion and magnetostriction experiments have been performed on a single crystal, in the temperature range from 5 K to room temperature. The YVO3 orders antiferromagnetically at T-N =
Ion-beam-assisted hexagonal diamond formation from C sub 6 sub 0 fullerene
Zhu, X D; Naramoto, H; Narumi, K; Miyashita, A; Miyashita, K
2003-01-01
Ions are commonly believed to be detrimental to diamond growth because of the high degree of lattice disorder induced by ion bombardments. In this paper, we examine the possibility of preparing diamond using thermally evaporated C sub 6 sub 0 and simultaneous bombardment with Ne sup + ions. It is found that the diamonds can be grown on Si wafers in the appropriate substrate temperature and ion energy ranges. Micro-Raman spectroscopy, x-ray diffractometry, and scanning electronic microscopy were employed to characterize the deposited specimen. These measurements provide definite evidence of the structure of nanosized hexagonal diamond. The mechanism responsible for the diamond formation is discussed.
Tetragonal phase of epitaxial room-temperature antiferromagnet CuMnAs.
Wadley, P; Novák, V; Campion, R P; Rinaldi, C; Martí, X; Reichlová, H; Zelezný, J; Gazquez, J; Roldan, M A; Varela, M; Khalyavin, D; Langridge, S; Kriegner, D; Máca, F; Mašek, J; Bertacco, R; Holý, V; Rushforth, A W; Edmonds, K W; Gallagher, B L; Foxon, C T; Wunderlich, J; Jungwirth, T
2013-01-01
Recent studies have demonstrated the potential of antiferromagnets as the active component in spintronic devices. This is in contrast to their current passive role as pinning layers in hard disk read heads and magnetic memories. Here we report the epitaxial growth of a new high-temperature antiferromagnetic material, tetragonal CuMnAs, which exhibits excellent crystal quality, chemical order and compatibility with existing semiconductor technologies. We demonstrate its growth on the III-V semiconductors GaAs and GaP, and show that the structure is also lattice matched to Si. Neutron diffraction shows collinear antiferromagnetic order with a high Néel temperature. Combined with our demonstration of room-temperature-exchange coupling in a CuMnAs/Fe bilayer, we conclude that tetragonal CuMnAs films are suitable candidate materials for antiferromagnetic spintronics.
Creation of an antiferromagnetic exchange spring
Scholl, A.; Liberati, M.; Arenholz, E.; Ohldag, H.; Stohr, J.
2004-04-06
We present evidence for the creation of an exchange spring in an antiferromagnet due to exchange coupling to a ferromagnet. X-ray magnetic linear dichroism spectroscopy on single crystal Co/NiO(001) shows that a partial domain wall is wound up at the surface of the antiferromagnet when the adjacent ferromagnet is rotated by a magnetic field. We determine the interface exchange stiffness and the antiferromagnetic domain wall energy from the field dependence of the direction of the antiferromagnetic axis, the antiferromagnetic pendant to a ferromagnetic hysteresis loop. The existence of a planar antiferromagnetic domain wall, proven by our measurement, is a key assumption of most exchange bias models.
Ullah, Mahtab, E-mail: mahtabullah@bzu.edu.pk [Department of Physics, Bahauddin Zakariya University Multan (Pakistan); Rana, Anwar Manzoor; Ahmad, E. [Department of Physics, Bahauddin Zakariya University Multan (Pakistan); Raza, Rizwan [Department of Physics, COMSATS Institute of Information Technology, Lahore-54000 (Pakistan); Hussain, Fayyaz [Department of Physics, Bahauddin Zakariya University Multan (Pakistan); Hussain, Akhtar; Iqbal, Muhammad [Theoretical Physics Division, PINSTECH, P.O. Nilore, Islamabad (Pakistan)
2016-09-01
Graphical abstract: - Highlights: • Fabrication of tantalum incorporated diamonds films using HFCVD technique. • Decrease in resistivity by increasing tantalum content in diamond thin films. • Electronic structure calculations of tantalum incorporated diamonds films through VASP code. • A rise of bond length and bond angles by addition of tantalum in the diamond lattice. • Confirmation of decrease of resistivity by adding tantalum due to creation of impurity states in the bandgap. - Abstract: Tantalum (Ta) incorporated diamond films are synthesized on silicon substrate by chemical vapor deposition under gas mixture of CH{sub 4} + H{sub 2}. Characterizations of the resulting films indicate that morphology and resistivity of as-grown diamond films are significantly influenced by the process parameters and the amount of tantalum incorporated in the diamond films. XRD plots reveal that diamond films are composed of TaC along with diamond for higher concentration of tantalum and Ta{sub 2}C phases for lower concentration of tantalum. EDS spectra confirms the existence of tantalum in the diamond films. Resistivity measurements illustrate a sudden fall of about two orders of magnitude by the addition of tantalum in the diamond films. Band structure of Ta-incorporated diamond has been investigated based on density functional theory (DFT) using VASP code. Band structure calculations lead to the semiconducting behavior of Ta-incorporated diamond films because of the creation of defects states inside the band gap extending towards conduction band minimum. Present DFT results support experimental trend of resistivity that with the incorporation of tantalum into diamond lattice causes a decrease in the resistivity of diamond films so that tantalum-incorporated diamond films behave like a good semiconductor.
Antiferromagnetic skyrmion crystals: Generation, topological Hall, and topological spin Hall effect
Göbel, Börge; Mook, Alexander; Henk, Jürgen; Mertig, Ingrid
2017-08-01
Skyrmions are topologically nontrivial, magnetic quasiparticles that are characterized by a topological charge. A regular array of skyrmions, a skyrmion crystal (SkX), features the topological Hall effect (THE) of electrons, which, in turn, gives rise to the Hall effect of the skyrmions themselves. It is commonly believed that antiferromagnetic skyrmion crystals (AFM-SkXs) lack both effects. In this Rapid Communication, we present a generally applicable method to create stable AFM-SkXs by growing a two-sublattice SkX onto a collinear antiferromagnet. As an example we show that both types of skyrmion crystals, conventional and antiferromagnetic, exist in honeycomb lattices. While AFM-SkXs with equivalent lattice sites do not show a THE, they exhibit a topological spin Hall effect. On top of this, AFM-SkXs on inequivalent sublattices exhibit a nonzero THE, which may be utilized in spintronics devices. Our theoretical findings call for experimental realization.
Hida, Kazuo
1992-03-01
The quantum disordered state (QDOS) of the spin 1/2 double layer square lattice Heisenberg antiferromagnet is studied. Using the dimer expansion from the limit of the large interlayer coupling J', the staggered susceptibility χ, the antiferromagnetic structure factor Sπ and the antiferromagnetic correlation length ξ are calculated up to the 6-th order in the intralayer coupling J. The ratio analysis shows that the QDOS becomes unstable against the Néel ordering at J'/J≃2.56. The critical exponents are not inconsistent with the universality class of the 3-dimensional classical Heisenberg model, suggesting that our QDOS corresponds to that expected in the 2-dimensional square lattice Heisenberg antiferromagnet with unphysically small spin (<0.276). The results of the projector Monte Carlo simulation also confirms the dimer expansion results.
STUDIES OF FCC HEISENBERG ANTIFERROMAGNETS BY MONTE CARLO SIMULATION ON LARGE SPIN ARRAYS
Minor, W.; Giebultowicz, T.
1988-01-01
We report Monte Carlo studies of fcc Heisenberg antiferromagnets carried out on arrays with 108,000 spins. A lattice with only JNN ≠ 0 was found to exhibit a Type I AF order despite the disordered nature of its ground state. Contrary to previous reports, our data indicate in this case a first order phase transition.
Neutron-scattering cross section of the S=1/2 Heisenberg triangular antiferromagnet
Lefmann, K.; Hedegård, P.
1994-01-01
In this paper we use a Schwinger-boson mean-field approach to calculate the neutron-scattering cross section from the S = 1/2 antiferromagnet with nearest-neighbor isotropic Heisenberg interaction on a two-dimensional triangular lattice. We investigate two solutions for T = 0: (i) a state with long...
Improved lower bounds on the ground-state entropy of the antiferromagnetic Potts model.
Chang, Shu-Chiuan; Shrock, Robert
2015-05-01
We present generalized methods for calculating lower bounds on the ground-state entropy per site, S(0), or equivalently, the ground-state degeneracy per site, W=e(S(0)/k(B)), of the antiferromagnetic Potts model. We use these methods to derive improved lower bounds on W for several lattices.
Thermophoresis of an antiferromagnetic soliton
Kim, Se Kwon; Tchernyshyov, Oleg; Tserkovnyak, Yaroslav
2015-07-01
We study the dynamics of an antiferromagnetic soliton under a temperature gradient. To this end, we start by phenomenologically constructing the stochastic Landau-Lifshitz-Gilbert equation for an antiferromagnet with the aid of the fluctuation-dissipation theorem. We then derive the Langevin equation for the soliton's center of mass by the collective coordinate approach. An antiferromagentic soliton behaves as a classical massive particle immersed in a viscous medium. By considering a thermodynamic ensemble of solitons, we obtain the Fokker-Planck equation, from which we extract the average drift velocity of a soliton. The diffusion coefficient is inversely proportional to a small damping constant α , which can yield a drift velocity of tens of m/s under a temperature gradient of 1 K/mm for a domain wall in an easy-axis antiferromagnetic wire with α ˜10-4 .
Schwandt, David; Mambrini, Matthieu; Poilblanc, Didier
2010-06-01
We propose a general nonperturbative scheme that quantitatively maps the low-energy sector of spin-1/2 frustrated Heisenberg antiferromagnets to effective generalized quantum dimer models. We develop the formal lattice-independent frame and establish some important results on (i) the locality of the generated Hamiltonians, (ii) how full resummations can be performed in this renormalization scheme. The method is then applied to the much debated kagome antiferromagnet for which a fully resummed effective Hamiltonian—shown to capture the essential properties and provide deep insights on the microscopic model [D. Poilblanc, M. Mambrini, and D. Schwandt, Phys. Rev. B 81, 180402(R) (2010)]—is derived.
Acoustic and optical phonons in metallic diamond
M. Hoesch, T. Fukuda, T. Takenouchi, J.P. Sutter, S. Tsutsui, A.Q.R. Baron, M. Nagao, Y. Takano, H. Kawarada and J. Mizuki
2006-01-01
Full Text Available The dispersion of acoustic and optical phonons in highly boron-doped diamond has been measured by inelastic X-ray scattering at an energy resolution of 6.4 meV. The sample is doped in the metallic regime and shows superconductivity below 4.2 K (midpoint. The data are compared to pure and nitrogen-doped diamond that represent the non-metallic state. No difference is found for the acoustic phonons in the three samples, while the optical phonons show a shift of the dispersion (softening in qualitative agreement with earlier results from Raman spectroscopy. The presence of boron and nitrogen incorporated into the diamond lattice leads to structural disorder. Evidence for this is found both in the observation of otherwise symmetry-forbidded Bragg intensity at (0 0 2 and intensity from acoustic phonon modes in the vicinity of (0 0 2.
Electronic structure studies of nanocrystalline diamond grain boundaries
Zapol, P.; Sternberg, M.; Frauenheim, T.; Gruen, D. M.; Curtiss, L. A.
1999-11-29
Diamond growth from hydrogen-poor plasmas results in diamond structures that are profoundly different from conventionally CVD-grown diamond. High concentration of carbon dimers in the microwave plasma results in a high rate of heterogeneous renucleation leading to formation of nanocrystalline diamond with a typical grain size of 3--10 nm. Therefore, up to 10% of carbon atoms are located in the grain boundaries. In this paper the authors report on density-functional based tight-binding molecular dynamics calculations of the structure of a {Sigma}13 twist (100) grain boundary in diamond. Beginning with a coincidence site lattice model, simulated annealing of the initial structure was performed at 1,500 K followed by relaxation toward lower temperatures. About one-half of the carbons in the grain boundary are found to be three-coordinated. Coordination numbers, bond length and bond angle distributions are analyzed and compared to those obtained in previous studies.
Superconductivity, antiferromagnetism, and neutron scattering
Tranquada, John M.; Xu, Guangyong; Zaliznyak, Igor A.
2014-01-01
High-temperature superconductivity in both the copper-oxide and the iron-pnictide/chalcogenide systems occurs in close proximity to antiferromagnetically ordered states. Neutron scattering has been an essential technique for characterizing the spin correlations in the antiferromagnetic phases and for demonstrating how the spin fluctuations persist in the superconductors. While the nature of the spin correlations in the superconductors remains controversial, the neutron scattering measurements of magnetic excitations over broad ranges of energy and momentum transfers provide important constraints on the theoretical options. We present an overview of the neutron scattering work on high-temperature superconductors and discuss some of the outstanding issues.
Watanabe, Tadataka; Hara, Shigeo; Ikeda, Shin-Ichi; Tomiyasu, Keisuke
2011-07-01
Ultrasound velocity measurements of the orbitally frustrated spinel GeCo2O4 reveal unique elastic anomalies within the antiferromagnetic phase. Temperature dependence of shear moduli exhibits a minimum within the antiferromagnetic phase, suggesting the coupling of shear acoustic phonons to molecular spin-orbit excitations. Magnetic-field dependence of elastic moduli exhibits diplike anomalies, being interpreted as magnetic-field-induced metamagnetic and structural transitions. These elastic anomalies suggest that the survival of geometrical frustration, and the interplay of spin, orbital, and lattice degrees of freedom evoke a set of phenomena in the antiferromagnetic phase.
Diamond heteroepitaxial lateral overgrowth
Tang, Yung-Hsiu
This dissertation describes improvements in the growth of single crystal diamond by microwave plasma-assisted chemical vapor deposition (CVD). Heteroepitaxial (001) diamond was grown on 1 cm. 2 a-plane sapphiresubstrates using an epitaxial (001) Ir thin-film as a buffer layer. Low-energy ion bombardment of the Ir layer, a process known as bias-enhanced nucleation, is a key step in achieving a high density of diamond nuclei. Bias conditions were optimized to form uniformly-high nucleation densities across the substrates, which led to well-coalesced diamond thin films after short growth times. Epitaxial lateral overgrowth (ELO) was used as a means of decreasing diamond internal stress by impeding the propagation of threading dislocations into the growing material. Its use in diamond growth requires adaptation to the aggressive chemical and thermal environment of the hydrogen plasma in a CVD reactor. Three ELO variants were developed. The most successful utilized a gold (Au) mask prepared by vacuum evaporation onto the surface of a thin heteroepitaxial diamond layer. The Au mask pattern, a series of parallel stripes on the micrometer scale, was produced by standard lift-off photolithography. When diamond overgrows the mask, dislocations are largely confined to the substrate. Differing degrees of confinement were studied by varying the stripe geometry and orientation. Significant improvement in diamond quality was found in the overgrown regions, as evidenced by reduction of the Raman scattering linewidth. The Au layer was found to remain intact during diamond overgrowth and did not chemically bond with the diamond surface. Besides impeding the propagation of threading dislocations, it was discovered that the thermally-induced stress in the CVD diamond was significantly reduced as a result of the ductile Au layer. Cracking and delamination of the diamond from the substrate was mostly eliminated. When diamond was grown to thicknesses above 0.1 mm it was found that
Revealing novel quantum phases in quantum antiferromagnets on random lattices
R. Yu
2009-01-01
Full Text Available Quantum magnets represent an ideal playground for the controlled realization of novel quantum phases and of quantum phase transitions. The Hamiltonian of the system can be indeed manipulated by applying a magnetic field or pressure on the sample. When doping the system with non-magnetic impurities, novel inhomogeneous phases emerge from the interplay between geometric randomness and quantum fluctuations. In this paper we review our recent work on quantum phase transitions and novel quantum phases realized in disordered quantum magnets. The system inhomogeneity is found to strongly affect phase transitions by changing their universality class, giving the transition a novel, quantum percolative nature. Such transitions connect conventionally ordered phases to unconventional, quantum disordered ones - quantum Griffiths phases, magnetic Bose glass phases - exhibiting gapless spectra associated with low-energy localized excitations.
Ferromagnetic and antiferromagnetic order in bacterial vortex lattices
Wioland, Hugo; Woodhouse, Francis G.; Dunkel, Jörn; Goldstein, Raymond E.
2016-01-01
This is the author accepted manuscript. The final version is available from Nature Publishing Group via http://dx.doi.org/10.1038/nphys3607 Despite their inherently non-equilibrium nature [1] , living systems can self-organize in highly ordered collective states [2,3] that share striking similarities with the thermodynamic equilibrium phases [4,5] of conventional condensed-matter and fluid systems. Examples range from the liquid-crystal-like arrangements of bacterial colonies [6,7], microb...
Fractional excitations in the square-lattice quantum antiferromagnet
Piazza, B. Dalla; Mourigal, M.; Christensen, Niels Bech
2015-01-01
Quantum magnets have occupied the fertile ground between many-body theory and low-temperature experiments on real materials since the early days of quantum mechanics. However, our understanding of even deceptively simple systems of interacting spin-1/2 particles is far from complete. The quantum ...
Diamond Synthesis Employing Nanoparticle Seeds
Uppireddi, Kishore (Inventor); Morell, Gerardo (Inventor); Weiner, Brad R. (Inventor)
2014-01-01
Iron nanoparticles were employed to induce the synthesis of diamond on molybdenum, silicon, and quartz substrates. Diamond films were grown using conventional conditions for diamond synthesis by hot filament chemical vapor deposition, except that dispersed iron oxide nanoparticles replaced the seeding. This approach to diamond induction can be combined with dip pen nanolithography for the selective deposition of diamond and diamond patterning while avoiding surface damage associated to diamond-seeding methods.
Symmetry Reduction in the Quantum Kagome Antiferromagnet Herbertsmithite
Zorko, A.; Herak, M.; Gomilšek, M.; van Tol, J.; Velázquez, M.; Khuntia, P.; Bert, F.; Mendels, P.
2017-01-01
Employing complementary torque magnetometry and electron spin resonance on single crystals of herbertsmithite, the closest realization to date of a quantum kagome antiferromagnet featuring a spin-liquid ground state, we provide novel insight into different contributions to its magnetism. At low temperatures, two distinct types of defects with different magnetic couplings to the kagome spins are found. Surprisingly, their magnetic response contradicts the threefold symmetry of the ideal kagome lattice, suggesting the presence of a global structural distortion that may be related to the establishment of the spin-liquid ground state.
Quenching the haldane gap in spin-1 Heisenberg antiferromagnets.
Wierschem, Keola; Sengupta, Pinaki
2014-06-20
We consider a quasi-one-dimensional system of spin-1 Heisenberg antiferromagnetic chains in two-dimensional and three-dimensional hypercubic lattices with interchain coupling J and uniaxial single-ion anisotropy D. Using large-scale numerical simulations, we map out the J-D phase diagram and investigate the low-lying excitations of the Haldane phase in the J≪1 limit. We also provide direct evidence that the Haldane phase remains a nontrivial symmetry-protected topological state for small but finite J.
Density matrix renormalization group numerical study of the kagome antiferromagnet.
Jiang, H C; Weng, Z Y; Sheng, D N
2008-09-12
We numerically study the spin-1/2 antiferromagnetic Heisenberg model on the kagome lattice using the density-matrix renormalization group method. We find that the ground state is a magnetically disordered spin liquid, characterized by an exponential decay of spin-spin correlation function in real space and a magnetic structure factor showing system-size independent peaks at commensurate magnetic wave vectors. We obtain a spin triplet excitation gap DeltaE(S=1)=0.055+/-0.005 by extrapolation based on the large size results, and confirm the presence of gapless singlet excitations. The physical nature of such an exotic spin liquid is also discussed.
Phase transitions in antiferromagnets with a NaCl structure
Kassan-Ogly, F.A. [Institute of Metal Physics, Ural Division, Russian Academy of Sciences, ul. S.Kovalevskoi 18, Ekaterinburg 620219 (Russian Federation)]. E-mail: felix.kassan-ogly@imp.uran.ru; Filippov, B.N. [Institute of Metal Physics, Ural Division, Russian Academy of Sciences, ul. S.Kovalevskoi 18, Ekaterinburg 620219 (Russian Federation)
2006-05-15
A revised derivation scheme of possible magnetic structures in an FCC lattice with the nearest- and next-nearest-neighbor interactions taken into account is proposed. A model of simultaneous magnetic and structural phase transitions of the first order is developed for antiferromagnets with a NaCl structure and with a strong cubic magnetic anisotropy on the base of synthesis of magnetic modified 6-state Potts model and theoretical models of structural phase transitions in cubic crystals. It is shown that the high-temperature diffuse magnetic scattering of neutrons transforms into magnetic Bragg reflections below Neel point.
Phase transitions in antiferromagnets with a NaCl structure
Kassan-Ogly, F. A.; Filippov, B. N.
2006-05-01
A revised derivation scheme of possible magnetic structures in an FCC lattice with the nearest- and next-nearest-neighbor interactions taken into account is proposed. A model of simultaneous magnetic and structural phase transitions of the first order is developed for antiferromagnets with a NaCl structure and with a strong cubic magnetic anisotropy on the base of synthesis of magnetic modified 6-state Potts model and theoretical models of structural phase transitions in cubic crystals. It is shown that the high-temperature diffuse magnetic scattering of neutrons transforms into magnetic Bragg reflections below Néel point.
Z2 antiferromagnetic topological insulators with broken C4 symmetry
Bègue, Frédéric; Pujol, Pierre; Ramazashvili, Revaz
2017-04-01
A two-dimensional topological insulator may arise in a centrosymmetric commensurate Néel antiferromagnet (AF), where staggered magnetization breaks both the elementary translation and time reversal, but retains their product as a symmetry. Fang et al. [6] proposed an expression for a Z2 topological invariant to characterize such systems. Here, we show that this expression does not allow to detect all the existing phases if a certain lattice symmetry is lacking. We implement numerical techniques to diagnose topological phases of a toy Hamiltonian, and verify our results by computing the Chern numbers of degenerate bands, and also by explicitly constructing the edge states, thus illustrating the efficiency of the method.
Chakrabarti, J; Bagchi, B; Chakrabarti, Jayprokas; Basu, Asis; Bagchi, Bijon
2000-01-01
Fermions on the lattice have bosonic excitations generated from the underlying periodic background. These, the lattice bosons, arise near the empty band or when the bands are nearly full. They do not depend on the nature of the interactions and exist for any fermion-fermion coupling. We discuss these lattice boson solutions for the Dirac Hamiltonian.
Diamond-cBN alloy: A universal cutting material
Wang, Pei [Institute of Atomic and Molecular Physics, Sichuan University, Chengdu 610065 (China); High Pressure Science and Engineering Center and Department of Physics and Astronomy, University of Nevada Las Vegas, Las Vegas, Nevada 89154 (United States); He, Duanwei, E-mail: duanweihe@scu.edu.cn; Kou, Zili; Li, Yong; Hu, Qiwei; Xu, Chao; Lei, Li; Wang, Qiming [Institute of Atomic and Molecular Physics, Sichuan University, Chengdu 610065 (China); Wang, Liping; Zhao, Yusheng [High Pressure Science and Engineering Center and Department of Physics and Astronomy, University of Nevada Las Vegas, Las Vegas, Nevada 89154 (United States); Xiong, Lun; Liu, Jing [Institute of High Energy Physics, Chinese Academy of Sciences, Beijing 100049 (China)
2015-09-07
Diamond and cubic boron nitride (cBN) as conventional superhard materials have found widespread industrial applications, but both have inherent limitations. Diamond is not suitable for high-speed cutting of ferrous materials due to its poor chemical inertness, while cBN is only about half as hard as diamond. Because of their affinity in structural lattices and covalent bonding character, diamond and cBN could form alloys that can potentially fill the performance gap. However, the idea has never been demonstrated because samples obtained in the previous studies were too small to be tested for their practical performance. Here, we report the synthesis and characterization of transparent bulk diamond-cBN alloy compacts whose diameters (3 mm) are sufficiently large for them to be processed into cutting tools. The testing results show that the diamond-cBN alloy has superior chemical inertness over polycrystalline diamond and higher hardness than single crystal cBN. High-speed cutting tests on hardened steel and granite suggest that diamond-cBN alloy is indeed a universal cutting material.
Nano-inclusions in diamond: Evidence of diamond genesis
Wirth, R.
2015-12-01
The use of Focused Ion Beam technology (FIB) for TEM sample preparation introduced approximately 15 years ago revolutionized the application of TEM in Geosciences. For the first time, FIB enabled cutting samples for TEM use from exactly the location we are interested in. Applied to diamond investigation, this technique revealed the presence of nanometre-sized inclusions in diamond that have been simply unknown before. Nanoinclusions in diamond from different location and origin such as diamonds from the Lower and Upper Mantle, metamorphic diamonds (Kazakhstan, Erzgebirge, Bohemia), diamonds from ophiolites (Tibet, Mongolia, Xinjiang, Ural Mountains), diamonds from igneous rocks (Hawaii, Kamchatka) and impact diamonds (Popigai Crater, Siberia) have been investigated during the last 15 years. The major conclusion of all these TEM studies is, that the nanoinclusions, their phases and phase composition together with the micro- and nanostructure evidence the origin of diamond and genesis of diamond. We can discriminate Five different mechanisms of diamond genesis in nature are observed: Diamond crystallized from a high-density fluid (Upper mantle and metamorphic diamond). Diamond crystallized from carbonatitic melt (Lower mantle diamond). Diamond precipitates from a metal alloy melt (Diamond from ophiolites). Diamond crystallized by gas phase condensation or chemical vapour condensation (CVD) (Lavas from Kamchatka, xenoliths in Hawaiian lavas). Direct transformation of graphite into diamond.
Large anomalous Hall effect in a half-Heusler antiferromagnet
Suzuki, T.; Chisnell, R.; Devarakonda, A.; Liu, Y.-T.; Feng, W.; Xiao, D.; Lynn, J. W.; Checkelsky, J. G.
2016-12-01
The quantum mechanical (Berry) phase of the electronic wavefunction plays a critical role in the anomalous and spin Hall effects, including their quantized limits. While progress has been made in understanding these effects in ferromagnets, less is known in antiferromagnetic systems. Here we present a study of antiferromagnet GdPtBi, whose electronic structure is similar to that of the topologically non-trivial HgTe (refs ,,), and where the Gd ions offer the possibility to tune the Berry phase via control of the spin texture. We show that this system supports an anomalous Hall angle ΘAH > 0.1, comparable to the largest observed in bulk ferromagnets and significantly larger than in other antiferromagnets. Neutron scattering measurements and electronic structure calculations suggest that this effect originates from avoided crossing or Weyl points that develop near the Fermi level due to a breaking of combined time-reversal and lattice symmetries. Berry phase effects associated with such symmetry breaking have recently been explored in kagome networks; our results extend this to half-Heusler systems with non-trivial band topology. The magnetic textures indicated here may also provide pathways towards realizing the topological insulating and semimetallic states predicted in this material class.
Neutron scattering studies of a frustrated spinel antiferromagnet in zero and high magnetic field
Matsuda, M [Quantum Beam Science Directorate, Japan Atomic Energy Agency (JAEA), Tokai, Ibaraki 319-1195 (Japan)
2006-11-15
A review is given of the neutron scattering studies on a frustrated spinel antiferromagnet CdCr{sub 2}O{sub 4}. As observed in ZnCr{sub 2}O{sub 4}, which has been most extensively studied in the Cr-based spinel oxides, CdCr{sub 2}O{sub 4} also shows an antiferromagnetic phase transition and a structural phase transition simultaneously, indicating a strong spin-lattice coupling. The magnetic structure of CdCr{sub 2}O{sub 4}was determined by neutron scattering studies. The neutron scattering study in magnetic field up to 10 T indicates an orientation of magnetic domains.
Zhang, N.G.; Henley, C.L.; Rischel, C.;
2002-01-01
We study the low-lying eigenenergy clustering patterns of quantum antiferromagnets with p sublattices (in particular p = 4). We treat each sublattice as a large spin, and using second-order degenerate perturbation theory, we derive the effective (biquadratic) Hamiltonian coupling the p large spins....... In order to compare with exact diagonalizations, the Hamiltonian is explicitly written for a finite-size lattice, and it contains information on energies of excited states as well as the ground state. The result is applied to the face-centered-cubic Type-I antiferromagnet of spin 1/2, including second...
Bond-Dilution Effects on Two-Dimensional Spin-Gapped Heisenberg Antiferromagnets
Yasuda, Chitoshi; Todo, Synge; Matsumoto, Munehisa; Takayama, Hajime
2001-01-01
Bond-dilution effects on spin-1/2 spin-gapped Heisenberg antiferromagnets of coupled alternating chains on a square lattice are investigated by means of the quantum Monte Carlo method. It is found that, in contrast with the site-diluted system having an infinitesimal critical concentration, the bond-diluted system has a finite critical concentration of diluted bonds, $x_{c}$, above which the system is in an antiferromagnetic (AF) long-range ordered phase. In the disordered phase below $x_{c}$...
Topological Weyl semimetals in the chiral antiferromagnetic materials Mn3Ge and Mn3Sn
Yang, Hao; Sun, Yan; Zhang, Yang; Shi, Wu-Jun; Parkin, Stuart S. P.; Yan, Binghai
2017-01-01
Recent experiments revealed that Mn3Sn and Mn3Ge exhibit a strong anomalous Hall effect at room temperature, provoking us to explore their electronic structures for topological properties. By ab initio band structure calculations, we have observed the existence of multiple Weyl points in the bulk and corresponding Fermi arcs on the surface, predicting antiferromagnetic Weyl semimetals in Mn3Ge and Mn3Sn. Here the chiral antiferromagnetism in the Kagome-type lattice structure is essential to determine the positions and numbers of Weyl points. Our work further reveals a new guiding principle to search for magnetic Weyl semimetals among materials that exhibit a strong anomalous Hall effect.
Giant electrothermal conductivity and spin-phonon coupling in an antiferromagnetic oxide.
Chiorescu, C; Neumeier, J J; Cohn, J L
2008-12-19
The application of weak electric fields ( less, similar 100 V/cm) is found to dramatically enhance the lattice thermal conductivity of the antiferromagnetic insulator CaMnO3 over a broad range of temperature about the Néel ordering point (125 K). The effect is coincident with field-induced detrapping of bound electrons, suggesting that phonon scattering associated with short- and long-ranged antiferromagnetic order is suppressed in the presence of the mobilized charge. This interplay between bound charge and spin-phonon coupling might allow for the reversible control of spin fluctuations using weak external fields.
Gammelmark, Søren; Eckardt, André
2013-01-01
We theoretically study the adiabatic preparation of an antiferromagnetic phase in a mixed Mott insulator of two bosonic atom species in a one-dimensional optical lattice. In such a system one can engineer a tunable parabolic inhomogeneity by controlling the difference of the trapping potentials...... felt by the two species. Using numerical simulations we predict that a finite parabolic potential can assist the adiabatic preparation of the antiferromagnet. The optimal strength of the parabolic inhomogeneity depends sensitively on the number imbalance between the two species. We also find...
Nonequilibrium antiferromagnetic mixed-spin Ising model.
Godoy, Mauricio; Figueiredo, Wagner
2002-09-01
We studied an antiferromagnetic mixed-spin Ising model on the square lattice subject to two competing stochastic processes. The model system consists of two interpenetrating sublattices of spins sigma=1/2 and S=1, and we take only nearest neighbor interactions between pairs of spins. The system is in contact with a heat bath at temperature T, and the exchange of energy with the heat bath occurs via one-spin flip (Glauber dynamics). Besides, the system interacts with an external agency of energy, which supplies energy to it whenever two nearest neighboring spins are simultaneously flipped. By employing Monte Carlo simulations and a dynamical pair approximation, we found the phase diagram for the stationary states of the model in the plane temperature T versus the competition parameter between one- and two-spin flips p. We observed the appearance of three distinct phases, that are separated by continuous transition lines. We also determined the static critical exponents along these lines and we showed that this nonequilibrium model belongs to the universality class of the two-dimensional equilibrium Ising model.
Antiferromagnetic Skyrmion: Stability, Creation and Manipulation
Zhang, Xichao; Zhou, Yan; Ezawa, Motohiko
2016-04-01
Magnetic skyrmions are particle-like topological excitations in ferromagnets, which have the topo-logical number Q = ± 1, and hence show the skyrmion Hall effect (SkHE) due to the Magnus force effect originating from the topology. Here, we propose the counterpart of the magnetic skyrmion in the antiferromagnetic (AFM) system, that is, the AFM skyrmion, which is topologically protected but without showing the SkHE. Two approaches for creating the AFM skyrmion have been described based on micromagnetic lattice simulations: (i) by injecting a vertical spin-polarized current to a nanodisk with the AFM ground state; (ii) by converting an AFM domain-wall pair in a nanowire junction. It is demonstrated that the AFM skyrmion, driven by the spin-polarized current, can move straightly over long distance, benefiting from the absence of the SkHE. Our results will open a new strategy on designing the novel spintronic devices based on AFM materials.
Landau model for the multiferroic delafossite antiferromagnets
Ribeiro, J.L, E-mail: jlr@fisica.uminho.pt [Centro de Física da Universidade do Minho, 4710-057 Braga (Portugal); Perez-Mato, J.M [Dpto. de Física de la Materia Condensada, Facultad de Ciencia y Tecnología, Universidad del País Vasco, Apartado 644, 48080 Bilbao (Spain); Vieira, L.G [Centro de Física da Universidade do Minho, 4710-057 Braga (Portugal)
2016-10-15
A symmetry based framework is used to describe the complex phase diagrams observed in the multiferroic delafossite compounds. A free energy Landau functional is derived from the analysis of the transformation properties of the most general incommensurate magnetic spin order parameter. A principle of maximal symmetry is invoked and the stability of each of the different higher symmetry phases considered. The competition between different potential ground states is analysed within the scope of a simplified model, which emphasizes the role of the symmetry allowed phase dependent biquadratic couplings. The cross-over between the different competing states is also discussed. The results show that the diverse set of phase diagrams that are experimentally observed in this class of triangular lattice antiferromagnets and, in particular, the stabilization of magnetically induced ferroelectric states, can be well interpreted and described within this integrated phenomenological approximation. - Highlights: • Symmetry considerations are used to analyze the phase diagrams of the compounds. • The competition between possible ground states is discussed. • The field induced transitions between competing states are described.
Diamond tool machining of materials which react with diamond
Lundin, Ralph L.; Stewart, Delbert D.; Evans, Christopher J.
1992-01-01
Apparatus for the diamond machining of materials which detrimentally react with diamond cutting tools in which the cutting tool and the workpiece are chilled to very low temperatures. This chilling halts or retards the chemical reaction between the workpiece and the diamond cutting tool so that wear rates of the diamond tool on previously detrimental materials are comparable with the diamond turning of materials which do not react with diamond.
Terada, N; Suzuki, H S; Kitazawa, H [National Institute for Materials Science (NIMS), Tsukuba, Ibaraki, 305-0047 (Japan); Kaneko, K; Metoki, N [Japan Atomic Energy Agency, Tokai, Ibaraki, 319-1195 (Japan); Awaka, J [National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba Central 5, 1-1-1 Higashi, Tsukuba, Ibaraki 305-8565 (Japan); Nagata, S, E-mail: terada.noriki@nims.go.j [Muroran Institute of Technology, 27-1 Mizumoto-cho, Muroran, Hokkaido, 050-8585 (Japan)
2010-01-01
We have investigated the magnetic orderings and the magnetic interactions in garnet antiferromagnets AgCa{sub 2}M{sub 2}V{sub 3}O{sub 12}(M=Mn, Co, Ni) and NaPb{sub 2}Mn{sub 2}V{sub 3}O{sub 12}, using the powder neutron diffraction and magnetization measurements. In the neutron diffraction measurements, we revealed that the magnetic structures in all samples measured are simple two sublattice antiferromagnetic structures with collinear magnetic moments. We also determined the exchange interactions from the critical magnetic fields H{sup sat} observed in the high field magnetization processes up to 30 T.
Optical engineering of diamond
Rabeau, James R
2013-01-01
This is the first comprehensive book on the engineering of diamond optical devices. It will give readers an up-to-date account of the properties of optical quality synthetic diamond (single crystal, nanodiamond and polycrystalline) and reviews the large and growing field of engineering of diamond-based optical devices, with applications in quantum computation, nano-imaging, high performance lasers, and biomedicine. It aims to provide scientists, engineers and physicists with a valuable resource and reference book for the design and performance of diamond-based optical devices.
Spin diffusion and torques in disordered antiferromagnets
Manchon, Aurelien
2017-02-01
We have developed a drift-diffusion equation of spin transport in collinear bipartite metallic antiferromagnets. Starting from a model tight-binding Hamiltonian, we obtain the quantum kinetic equation within Keldysh formalism and expand it to the lowest order in spatial gradient using Wigner expansion method. In the diffusive limit, these equations track the spatio-temporal evolution of the spin accumulations and spin currents on each sublattice of the antiferromagnet. We use these equations to address the nature of the spin transfer torque in (i) a spin-valve composed of a ferromagnet and an antiferromagnet, (ii) a metallic bilayer consisting of an antiferromagnet adjacent to a heavy metal possessing spin Hall effect, and in (iii) a single antiferromagnet possessing spin Hall effect. We show that the latter can experience a self-torque thanks to the non-vanishing spin Hall effect in the antiferromagnet.
Thermoinduced magnetization in nanoparticles of antiferromagnetic materials
Mørup, Steen; Frandsen, Cathrine
2004-01-01
We show that there is a thermoinduced contribution to the magnetic moment of nanoparticles of antiferromagnetic materials. It arises from thermal excitations of the uniform spin-precession mode, and it has the unusual property that its magnitude increases with increasing temperature. This has...... the consequence that antiferromagnetism is nonexistent in nanoparticles at finite temperatures and it explains magnetic anomalies, which recently have been reported in a number of studies of nanoparticles of antiferromagnetic materials....
Yarash K. Abuev
2017-01-01
Full Text Available Abstract. Objectives A computer simulation of the antiferromagnetic structures described by the three-vertex Potts model on a triangular lattice is performed, taking into account the antiferromagnetic exchange interactions between the nearest J1 and second J2 neighbours. The main goal of the computer simulation was to elucidate the effects of ground state and areas of frustration on the thermodynamic and magnetic properties of antiferromagnetic structures described by the lowdimensional Potts model. Method The computer simulation is based on the Monte Carlo method. This method is implemented using the Metropolis algorithm in combination with the Wolff claster algorithm. The computer simulation was carried out for low-dimensional systems with periodic boundary conditions and linear dimensions L = 24124. Results On the basis of heat capacity and entropy analysis, phase transitions were observed in the considered model to possess exchange interaction parameters J1 <0 and J2 <0 in the variation intervals 0r<0.2 and 1.0
Large magnetostriction and negative thermal expansion in the frustrated antiferromagnet ZnCr2Se4.
Hemberger, J; von Nidda, H-A Krug; Tsurkan, V; Loidl, A
2007-04-06
A detailed investigation of ZnCr2Se4 is presented which is dominated by strong ferromagnetic exchange but orders antiferromagnetically at TN=21 K. Specific heat and thermal expansion exhibit sharp first-order anomalies at the antiferromagnetic transition. TN is shifted to lower temperatures by external magnetic fields and finally is fully suppressed by a field of 65 kOe. The relative length change DeltaL/L(T) is unusually large and exhibits negative thermal expansion alpha below 75 K down to TN indicating strong frustration of the lattice. Magnetostriction DeltaL/L(H) reveals large values comparable to giant magnetostrictive materials. These results point to a spin-driven origin of the structural instability at TN explained in terms of competing ferromagnetic and antiferromagnetic exchange interactions.
Relativistic Néel-Order Fields Induced by Electrical Current in Antiferromagnets
Železný, J.
2014-10-06
We predict that a lateral electrical current in antiferromagnets can induce nonequilibrium Néel-order fields, i.e., fields whose sign alternates between the spin sublattices, which can trigger ultrafast spin-axis reorientation. Based on microscopic transport theory calculations we identify staggered current-induced fields analogous to the intraband and to the intrinsic interband spin-orbit fields previously reported in ferromagnets with a broken inversion-symmetry crystal. To illustrate their rich physics and utility, we consider bulk Mn2Au with the two spin sublattices forming inversion partners, and a 2D square-lattice antiferromagnet with broken structural inversion symmetry modeled by a Rashba spin-orbit coupling. We propose an antiferromagnetic memory device with electrical writing and reading.
Indications of c-axis Charge Transport in Hole Doped Triangular Antiferromagnets
LIANG Ying; LIU Bin; FENG Shi-Ping
2004-01-01
The c-axis charge transport of the hole doped triangular antiferromagnet is investigated within the tJ model by considering the incoherent interlayer hopping.It is shown that the c-axis charge transport of the hole doped triangular antiferromagnet is essentially determined by the scattering from the in-plane fluctuation.The c-axis conductivity spectrum shows a lov-energy peak and the unusual high-energy broad band,while the c-axis resistivity is characterized by a crossover from the high temperature metallic-like behavior to the Iow temperature insulating-like behavior,which is qualitatively consistent with those of the hole doped square lattice antiferromagnet.
Nuclear techniques of analysis in diamond synthesis and annealing
Jamieson, D. N.; Prawer, S.; Gonon, P.; Walker, R.; Dooley, S.; Bettiol, A.; Pearce, J. [Melbourne Univ., Parkville, VIC (Australia). School of Physics
1996-12-31
Nuclear techniques of analysis have played an important role in the study of synthetic and laser annealed diamond. These measurements have mainly used ion beam analysis with a focused MeV ion beam in a nuclear microprobe system. A variety of techniques have been employed. One of the most important is nuclear elastic scattering, sometimes called non-Rutherford scattering, which has been used to accurately characterise diamond films for thickness and composition. This is possible by the use of a database of measured scattering cross sections. Recently, this work has been extended and nuclear elastic scattering cross sections for both natural boron isotopes have been measured. For radiation damaged diamond, a focused laser annealing scheme has been developed which produces near complete regrowth of MeV phosphorus implanted diamonds. In the laser annealed regions, proton induced x-ray emission has been used to show that 50 % of the P atoms occupy lattice sites. This opens the way to produce n-type diamond for microelectronic device applications. All these analytical applications utilize a focused MeV microbeam which is ideally suited for diamond analysis. This presentation reviews these applications, as well as the technology of nuclear techniques of analysis for diamond with a focused beam. 9 refs., 6 figs.
Diamond films: Historical perspective
Messier, R. [Pennsylvania State Univ., University Park (United States)
1993-01-01
This section is a compilation of notes and published international articles about the development of methods of depositing diamond films. Vapor deposition articles are included from American, Russian, and Japanese publications. The international competition to develop new deposition methodologies is stressed. The current status of chemical vapor deposition of diamond is assessed.
Renneboog, Luc
2015-01-01
This paper examines the risk-return characteristics of investment grade gems (white diamonds, colored diamonds and other types of gems including sapphires, rubies, and emeralds). The transactions are coming from gem auctions and span the period 1999-2012. Over our time frame, the annual nominal USD
Renneboog, Luc
2015-01-01
This paper examines the risk-return characteristics of investment grade gems (white diamonds, colored diamonds and other types of gems including sapphires, rubies, and emeralds). The transactions are coming from gem auctions and span the period 1999-2012. Over our time frame, the annual nominal USD
Motome, Yukitoshi; Penc, Karlo; Shannon, Nic
2005-01-01
The antiferromagnetic Heisenberg model on a pyrochlore lattice under external magnetic field is studied by classical Monte Carlo simulation. The model includes bilinear and biquadratic interactions; the latter effectively describes the coupling to lattice distortions. The magnetization process shows a half-magnetization plateau at low temperatures, accompanied with strong suppression of the magnetic susceptibility. Temperature dependence of the plateau behavior is clarified. Finite-temperatur...
Yury Gutsalenko
2010-06-01
Full Text Available The paper generalizes on the one hand theory of kinematic-geometrical simulation of grinding processes by means of tools with working part as binding matrix with abrasive grains located in it in random manner, for example diamond grains, and on the other hand practical performance of combined grinding process, based on introduction of additional energy as electric discharges and called by the organization-developer (Kharkov Polytechnic Institute «diamond-spark grinding» as applied to processing by means of diamond wheel. Implementation of diamond-spark grinding technologies on the basis of developed generalized theoretical approach allows to use the tool with prescribed tool-life, moreover to make the most efficient use of it up to full exhausting of tool-life, determined by diamond-bearing thickness. Development is directed forward computer-aided manufacturing.
Diamond Integrated Optomechanical Circuits
Rath, Patrik; Nebel, Christoph; Wild, Christoph; Pernice, Wolfram H P
2013-01-01
Diamond offers unique material advantages for the realization of micro- and nanomechanical resonators due to its high Young's modulus, compatibility with harsh environments and superior thermal properties. At the same time, the wide electronic bandgap of 5.45eV makes diamond a suitable material for integrated optics because of broadband transparency and the absence of free-carrier absorption commonly encountered in silicon photonics. Here we take advantage of both to engineer full-scale optomechanical circuits in diamond thin films. We show that polycrystalline diamond films fabricated by chemical vapour deposition provide a convenient waferscale substrate for the realization of high quality nanophotonic devices. Using free-standing nanomechanical resonators embedded in on-chip Mach-Zehnder interferometers, we demonstrate efficient optomechanical transduction via gradient optical forces. Fabricated diamond resonators reproducibly show high mechanical quality factors up to 11,200. Our low cost, wideband, carri...
Quasiparticle excitations in frustrated antiferromagnets
Trumper, Adolfo E. [Instituto de Fisica Rosario (CONICET) Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina)]. E-mail: trumper@ifir.edu.ar; Gazza, Claudio J. [Instituto de Fisica Rosario (CONICET) Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina); Manuel, Luis O. [Instituto de Fisica Rosario (CONICET) Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina)]. E-mail: manuel@ifir.edu.ar
2004-12-31
We have computed the quasiparticle wave function corresponding to a hole injected in a triangular antiferromagnet. We have taken into account multi-magnon contributions within the self-consistent Born approximation. We have found qualitative differences, under sign reversal of the integral transfer t, regarding the multi-magnon components and the own existence of the quasiparticle excitations. Such differences are due to the subtle interplay between magnon-assisted and free hopping mechanisms. We conclude that the conventional quasiparticle picture can be broken by geometrical frustration without invoking spin liquid phases.
Wang, Da-Wei; Zhu, Shi-Yao; Scully, Marlan O
2014-01-01
We show that the timed Dicke states of a collection of three-level atoms can form a tight-binding lattice in the momentum space. This lattice, coined the superradiance lattice (SL), can be constructed based on an electromagnetically induced transparency (EIT) system. For a one-dimensional SL, we need the coupling field of the EIT system to be a standing wave. The detuning between the two components of the standing wave introduces an effective electric field. The quantum behaviours of electrons in lattices, such as Bloch oscillations, Wannier-Stark ladders, Bloch band collapsing and dynamic localization can be observed in the SL. The SL can be extended to two, three and even higher dimensions where no analogous real space lattices exist and new physics are waiting to be explored.
Ionoluminescence of diamond, synthetic diamond and simulants
Calvo del Castillo, H. [Departamento de Geologia y Geoquimica, Facultad de Ciencias, Universidad Autonoma de Madrid, Ctra de Colmenar km 15, Madrid 27049 (Spain); Instituto de Fisica, Universidad Nacional Autonoma de Mexico, Circuito de la Investigacion Cientifica s/n, Ciudad Universitaria, Ciudad de Mexico 04519, Mexico, DF (Mexico); Ruvalcaba-Sil, J.L. [Instituto de Fisica, Universidad Nacional Autonoma de Mexico, Circuito de la Investigacion Cientifica s/n, Ciudad Universitaria, Ciudad de Mexico 04519, Mexico, DF (Mexico); Barboza-Flores, M. [Centro de Investigacio en Fisica, Universidad de Sonora, Apartado postal 5-088, Hermosillo, Sonora 83190 (Mexico); Belmont, E. [Instituto de Fisica, Universidad Nacional Autonoma de Mexico, Circuito de la Investigacion Cientifica s/n, Ciudad Universitaria, Ciudad de Mexico 04519, Mexico, DF (Mexico); Calderon, T. [Departamento de Geologia y Geoquimica, Facultad de Ciencias, Universidad Autonoma de Madrid, Ctra de Colmenar km 15, Madrid 27049 (Spain)], E-mail: tomas.calderon@uam.es
2007-09-21
Ionoluminescence (IL) spectra of diamond (natural samples and synthetic CVD) and its more common synthetic simulates such as sapphire, spinel, cubic zirconia, strontium titanate and yttrium aluminium garnet (YAG: Er) will be discussed here in order to support some criteria that will allow to distinguish between them. While diamond shows emission bands due to nitrogen defects, simulants feature d-transition metals and rare earths such as Cr{sup 3+}, Mn{sup 2+}, Fe{sup 3+}, Ti{sup 3+} and Er{sup 3+} emissions.
Spin dynamics in charge doped antiferromagnets : a Li-7 NMR study in Ni1-xLixO
Tedoldi, F; Marini, S; Corti, M
1997-01-01
The effects of heterovalent substitutions causing itinerant holes in strongly correlated 3d electron systems are studied by means of Li-7 NMR in lithium-doped antiferromagnetic NiO. The spin-lattice relaxation rates, driven by the fluctuation of Ni2+ (S = 1) ions, in the temperature range 10 K
Magnetic correlations in the 2D S=5/2 honeycomb antiferromagnet MnPS_{3}
Rønnow, H.M.; Wildes, A.R.; Bramwell, S.T.
2000-01-01
MnPS3 is a quasi-2D S = 5/2 antiferromagnet on a honeycomb lattice. Using an energy integrating neutron scattering technique, we have measured the structure factor S(k) of the instantaneous magnetic fluctuations. The temperature dependence of the correlation length xi follows the Kosterlitz...
Spin dynamics in charge doped antiferromagnets : a Li-7 NMR study in Ni1-xLixO
Tedoldi, F; Marini, S; Corti, M
1997-01-01
The effects of heterovalent substitutions causing itinerant holes in strongly correlated 3d electron systems are studied by means of Li-7 NMR in lithium-doped antiferromagnetic NiO. The spin-lattice relaxation rates, driven by the fluctuation of Ni2+ (S = 1) ions, in the temperature range 10 K
Spin dynamics in charge doped antiferromagnets : a Li-7 NMR study in Ni1-xLixO
Tedoldi, F; Marini, S; Corti, M
1997-01-01
The effects of heterovalent substitutions causing itinerant holes in strongly correlated 3d electron systems are studied by means of Li-7 NMR in lithium-doped antiferromagnetic NiO. The spin-lattice relaxation rates, driven by the fluctuation of Ni2+ (S = 1) ions, in the temperature range 10 K
Zitzler, R.; Pruschke, Th.; Bulla, R.
2004-05-01
We discuss the magnetic phase diagram for the Hubbard model with magnetic frustration obtained within the dynamical mean-field theory. Most interesting is the appearance of a first-order paramagnetic metal to antiferromagnetic insulator transition for the magnetically frustrated lattice at half filling. For finite doping the antiferromagnetic phase is susceptible to phase separation and competes with an itinerant ferromagnetic phase (Nagaoka ferromagnetism), leading to an unexpectedly rich magnetic phase diagram.
Zitzler, R.; Pruschke, Th. E-mail: pruschke@theorie.physik.uni-goettingen.de; Bulla, R
2004-05-01
We discuss the magnetic phase diagram for the Hubbard model with magnetic frustration obtained within the dynamical mean-field theory. Most interesting is the appearance of a first-order paramagnetic metal to antiferromagnetic insulator transition for the magnetically frustrated lattice at half filling. For finite doping the antiferromagnetic phase is susceptible to phase separation and competes with an itinerant ferromagnetic phase (Nagaoka ferromagnetism), leading to an unexpectedly rich magnetic phase diagram.
Purely antiferromagnetic magnetoelectric random access memory
Kosub, Tobias; Kopte, Martin; Hühne, Ruben; Appel, Patrick; Shields, Brendan; Maletinsky, Patrick; Hübner, René; Liedke, Maciej Oskar; Fassbender, Jürgen; Schmidt, Oliver G.; Makarov, Denys
2017-01-01
Magnetic random access memory schemes employing magnetoelectric coupling to write binary information promise outstanding energy efficiency. We propose and demonstrate a purely antiferromagnetic magnetoelectric random access memory (AF-MERAM) that offers a remarkable 50-fold reduction of the writing threshold compared with ferromagnet-based counterparts, is robust against magnetic disturbances and exhibits no ferromagnetic hysteresis losses. Using the magnetoelectric antiferromagnet Cr2O3, we demonstrate reliable isothermal switching via gate voltage pulses and all-electric readout at room temperature. As no ferromagnetic component is present in the system, the writing magnetic field does not need to be pulsed for readout, allowing permanent magnets to be used. Based on our prototypes, we construct a comprehensive model of the magnetoelectric selection mechanisms in thin films of magnetoelectric antiferromagnets, revealing misfit induced ferrimagnetism as an important factor. Beyond memory applications, the AF-MERAM concept introduces a general all-electric interface for antiferromagnets and should find wide applicability in antiferromagnetic spintronics.
Phase transition in Heisenberg stacked triangular antiferromagnets: end of a controversy.
Ngo, V Thanh; Diep, H T
2008-09-01
By using the Wang-Landau flat-histogram Monte Carlo (MC) method for very large lattice sizes never simulated before, we show that the phase transition in the frustrated Heisenberg stacked triangular antiferromagnet is of first order, contrary to results of earlier MC simulations using old-fashioned methods. Our result lends support to the conclusion of a nonperturbative renormalization group performed on an effective Hamiltonian. It puts an end to a 20-year -long controversial issue.
Yasuda, Shinya; Todo, Synge
2013-12-01
We present a method that optimizes the aspect ratio of a spatially anisotropic quantum lattice model during the quantum Monte Carlo simulation, and realizes the virtually isotropic lattice automatically. The anisotropy is removed by using the Robbins-Monro algorithm based on the correlation length in each direction. The method allows for comparing directly the value of the critical amplitude among different anisotropic models, and identifying the universality more precisely. We apply our method to the staggered dimer antiferromagnetic Heisenberg model and demonstrate that the apparent nonuniversal behavior is attributed mainly to the strong size correction of the effective aspect ratio due to the existence of the cubic interaction.
Z Jalali mola
2011-12-01
Full Text Available The Ising model is one of the simplest models describing the interacting particles. In this work, we calculate the high temperature series expansions of zero field susceptibility of ising model with ferromagnetic, antiferromagnetic and one antiferromagnetic interactions on two dimensional kagome lattice. Using the Pade´ approximation, we calculate the susceptibility of critical exponent of ferromagnetic ising model γ ≈ 1.75, which is consistent with universality hypothesis. However, antiferromagnetic and one antiferromagnetic interaction ising model doesn’t show any transition at finite temperature because of the effect of magnetic frustration.
Hamza, Alex V.; Biener, Juergen; Wild, Christoph; Woerner, Eckhard
2016-11-01
A novel method for fabricating diamond shells is introduced. The fabrication of such shells is a multi-step process, which involves diamond chemical vapor deposition on predetermined mandrels followed by polishing, microfabrication of holes, and removal of the mandrel by an etch process. The resultant shells of the present invention can be configured with a surface roughness at the nanometer level (e.g., on the order of down to about 10 nm RMS) on a mm length scale, and exhibit excellent hardness/strength, and good transparency in the both the infra-red and visible. Specifically, a novel process is disclosed herein, which allows coating of spherical substrates with optical-quality diamond films or nanocrystalline diamond films.
Functionalized diamond nanoparticles
Beaujuge, Pierre M.
2014-10-21
A diamond nanoparticle can be functionalized with a substituted dienophile under ambient conditions, and in the absence of catalysts or additional reagents. The functionalization is thought to proceed through an addition reaction.
Diamond nanobeam waveguide optomechanics
Khanaliloo, Behzad; Hryciw, Aaron C; Lake, David P; Kaviani, Hamidreza; Barclay, Paul E
2015-01-01
Optomechanical devices sensitively transduce and actuate motion of nanomechanical structures using light, and are central to many recent fundamental studies and technological advances. Single--crystal diamond promises to improve the performance of optomechanical devices, while also providing opportunities to interface nanomechanics with diamond color center spins and related quantum technologies. Here we demonstrate measurement of diamond nanobeam resonators with a sensitivity of 9.5 fm/Hz^0.5 and bandwidth >120 nm through dissipative waveguide--optomechanical coupling. Nanobeams are fabricated from bulk single--crystal diamond using a scalable quasi--isotropic oxygen plasma undercut etching process, and support mechanical resonances with quality factor of 2.5 x 10^5 at room temperature, and 7.2 x 10^5 in cryogenic conditions (5K). Mechanical self--oscillations, resulting from interplay between optomechanical coupling and the photothermal response of nanobeams in a buckled state, are observed with amplitude e...
Quantum engineering: Diamond envy
Nunn, Joshua
2013-03-01
Nitrogen atoms trapped tens of nanometres apart in diamond can now be linked by quantum entanglement. This ability to produce and control entanglement in solid systems could enable powerful quantum computers.
Femtosecond optomagnetism in dielectric antiferromagnets
Bossini, D.; Rasing, Th
2017-02-01
Optical femtosecond manipulation of magnetic order is attractive for the development of new concepts for ultrafast magnetic recording. Theoretical and experimental investigations in this research area aim at establishing a physical understanding of magnetic media in light-induced non-equilibrium states. Such a quest requires one to adjust the theory of magnetism, since the thermodynamical concepts of elementary excitations and spin alignment determined by the exchange interaction are not applicable on the femtosecond time-scale after the photo-excitation. Here we report some key milestones concerning the femtosecond optical control of spins in dielectric antiferromagnets, whose spin dynamics is by nature faster than that of ferromagnets and can be triggered even without any laser heating. The recent progress of the opto-magnetic effect in the sub-wavelength regime makes this exciting research area even more promising, in terms of both fundamental breakthroughs and technological perspectives.
Antiferromagnetic topological nodal line semimetals
Wang, Jing
2017-08-01
We study three-dimensional nodal line semimetals (NLSMs) with magnetic ordering and strong spin-orbit interaction. Two distinct classes of magnetic NLSMs are proposed. The first class is band-inversion NLSM where the accidental line node is induced by band inversion and locally protected by glide mirror plane and the combined time-reversal and inversion symmetries. This can be viewed as a trivial stacking of the two-dimensional antiferromagnetic Dirac semimetals. The second class is essential NLSM where the nodal features are filling enforced by specific magnetic symmetry group. We further provide two concrete tight-binding models for magnetic NLSMs which belong to these two different classes, respectively. We conclude with a brief discussion on the possible material venues and the experimental implications for such phases.
Bubnov, Igor N.; Falkovych, I. S.; Gridin, A. A.; Stanislavsky, A. A.; Reznik, A. P.
2015-01-01
Advantages of the diamond dipole antenna as an active antenna are presented. Such an antenna is like an inverted bow-tie antenna, but the former has some advantages over the ordinary bow-tie antenna. It is shown that the diamond dipole antenna may be an effective element of a new antenna array for low-frequency radio astronomy as well as a communication antenna.
Striped spin liquid crystal ground state instability of kagome antiferromagnets.
Clark, Bryan K; Kinder, Jesse M; Neuscamman, Eric; Chan, Garnet Kin-Lic; Lawler, Michael J
2013-11-01
The Dirac spin liquid ground state of the spin 1/2 Heisenberg kagome antiferromagnet has potential instabilities. This has been suggested as the reason why it does not emerge as the ground state in large-scale numerical calculations. However, previous attempts to observe these instabilities have failed. We report on the discovery of a projected BCS state with lower energy than the projected Dirac spin liquid state which provides new insight into the stability of the ground state of the kagome antiferromagnet. The new state has three remarkable features. First, it breaks spatial symmetry in an unusual way that may leave spinons deconfined along one direction. Second, it breaks the U(1) gauge symmetry down to Z(2). Third, it has the spatial symmetry of a previously proposed "monopole" suggesting that it is an instability of the Dirac spin liquid. The state described herein also shares a remarkable similarity to the distortion of the kagome lattice observed at low Zn concentrations in Zn-paratacamite and in recently grown single crystals of volborthite suggesting it may already be realized in these materials.
Magnetocaloric properties of a frustrated Blume-Capel antiferromagnet
Žukovič Milan
2014-07-01
Full Text Available Low-temperature magnetization processes and magnetocaloric properties of a geometrically frustrated spin-1 Blume-Capel model on a triangular lattice are studied by Monte Carlo simulations. The model is found to display qualitatively different behavior depending on the sign of the single-ion anisotropy D. For positive values of D we observe two magnetization plateaus, similar to the spin-1/2 Ising antiferromagnet, and negative isothermal entropy changes for any field intensity. For a range of small negative values of D there are four magnetization plateaus and the entropy changes can be either negative or positive, depending on the field. If D is negative but large in absolute value then the entropy changes are solely positive.
Terahertz-Driven Nonlinear Spin Response of Antiferromagnetic Nickel Oxide
Baierl, S.; Mentink, J. H.; Hohenleutner, M.; Braun, L.; Do, T.-M.; Lange, C.; Sell, A.; Fiebig, M.; Woltersdorf, G.; Kampfrath, T.; Huber, R.
2016-11-01
Terahertz magnetic fields with amplitudes of up to 0.4 Tesla drive magnon resonances in nickel oxide while the induced dynamics is recorded by femtosecond magneto-optical probing. We observe distinct spin-mediated optical nonlinearities, including oscillations at the second harmonic of the 1 THz magnon mode. The latter originate from coherent dynamics of the longitudinal component of the antiferromagnetic order parameter, which are probed by magneto-optical effects of second order in the spin deflection. These observations allow us to dynamically disentangle electronic from lattice-related contributions to magnetic linear birefringence and dichroism—information so far only accessible by ultrafast THz spin control. The nonlinearities discussed here foreshadow physics that will become essential in future subcycle spin switching.
Space Group Symmetry Fractionalization in a Chiral Kagome Heisenberg Antiferromagnet.
Zaletel, Michael P; Zhu, Zhenyue; Lu, Yuan-Ming; Vishwanath, Ashvin; White, Steven R
2016-05-13
The anyonic excitations of a spin liquid can feature fractional quantum numbers under space group symmetries. Detecting these fractional quantum numbers, which are analogs of the fractional charge of Laughlin quasiparticles, may prove easier than the direct observation of anyonic braiding and statistics. Motivated by the recent numerical discovery of spin-liquid phases in the kagome Heisenberg antiferromagnet, we theoretically predict the pattern of space group symmetry fractionalization in the kagome lattice SO(3)-symmetric chiral spin liquid. We provide a method to detect these fractional quantum numbers in finite-size numerics which is simple to implement in the density matrix renormalization group. Applying these developments to the chiral spin liquid phase of a kagome Heisenberg model, we find perfect agreement between our theoretical prediction and numerical observations.
Magnetic Orders and Fluctuations in the Dipolar Pyrochlore Antiferromagnet
Cepas, Olivier; Shastry, B. Sriram
2005-03-01
While the classical Heisenberg antiferromagnet on the pyrochlore lattice does not order, we will discuss, from a theoretical standpoint, possible magnetic phases induced by the dipole-dipole interactions. Such interactions play a role in systems such as Gd2Ti2O7 or Gd2Sn2O7 in stabilizing exotic forms of magnetic order, a subject of current debate. We will also argue that the external magnetic field induces multiple transitions, one of which is associated with no obvious broken symmetry, but can be characterized by a disorder parameter. Finally, Monte-Carlo simulations and Landau-Ginzburg expansion show that the dipolar Heisenberg model exhibits a fluctuation-induced first-order transition, thanks to the frustration and a continuous set of soft modes.
Potassium tantalate substrates for neutron experiments on antiferromagnetic perovskite films
Christen, H M; MacDougall, G J; Kim, H-S; Kim, D H; Boatner, L A; Bennett, C J Callender; Zarestky, J L; Nagler, S E, E-mail: christenhm@ornl.gov
2010-11-01
For the study of antiferromagnetism in thin-film materials, neutron diffraction is a particularly important tool, especially since magnetometry experiments are often complicated by the substrate's strong diamagnetic or paramagnetic contribution. However, the substrate, by necessity, has a lattice parameter that is very similar to that of the film, and in most cases is over 1000 times more massive than the film. Therefore, even weak structural distortions in the substrate crystal may complicate the analysis of magnetic scattering from the film. Here we show that in contrast to most other perovskite substrates (including SrTiO{sub 3}, LaAlO{sub 3}, etc.), KTaO3 provides a uniquely appropriate substrate platform for magnetic diffraction experiments on epitaxial oxide films.
Spin-phonon interaction in antiferromagnetics
Grigorashchuk, I.M.; Nitsovich, V.M.; Tovstyuk, K.D.
1975-01-01
The vibrational spectrum and the sound velocity in antiferromagnetics are obtained in the general form in pseudoharmonic approximation with allowance for the anharmonisms of all orders. Starting from experimentally defined dependence of the Debye-Waller factor on the temperature a corollary is put forward that in some antiferromagnetics under the temperature lower than T/subN/ the appearance of the narrow band of paramagnetic states is possible. In antiferromagnetics where the transition metal-dielectric described by the Habbard model is possible this results in the appearance of the additional transition dielectric-metal-dielectric. (auth)
High Precision Calculations of the Lennard-Jones Lattice Constants for Five Lattices
Stein, Matthew
2017-01-01
The total potential energy of a crystal as described by the Lennard-Jones (L-J) potential depends in part upon the calculation of lattice constants. Knowing these constants to high precision is useful for prediction of the lattice type and simulation of crystals such as rare-gas solids or germanium detectors, but reaching higher precision is computationally costly and challenging. Presented here is the extension of the precision of the lattice constants, Lp, up to 32 decimal digits, and in some cases corrections from previous publication. The Lp terms are given for 4 cubic, face-centered cubic, body-centered cubic, hexagonal-close-pack, and diamond lattices. This precision was obtained through the use of careful parallelization technique, exploitation of the symmetries of each lattice, and the ``onionization'' of the simulated crystal. The results of this computation, along with the tools and algorithm strategies to make this computation possible, are explained in detail graphically.
Hu Jing-Guo; Stamps R L
2006-01-01
The rotational anisotropies in the exchange bias structures of ferromagnetism/antiferromagnetism 1/antiferromagnetism 2 are studied in this paper. Based on the model, in which the antiferromagnetism is treated with an Ising mean field theory and the rotational anisotropy is assumed to be related to the field created by the moment induced on the antiferromagnetic layer next to the ferromagnetic layer, we can explain why in experiments for ferromagnetism (FM)/antiferromagntism 1 (AFM1)/antiferromagnetism 2 (AFM2) systems the thickness-dependent rotational anisotropy value is non-monotonic, i.e. it reaches a minimum for this system at a specific thickness of the first antiferromagnetic layer and exhibits oscillatory behaviour. In addition, we find that the temperature-dependent rotational anisotropy value is in good agreement with the experimental result.
Cryotribology of diamond and graphite
Iwasa, Yukikazu; Ashaboglu, A.F.; Rabinowicz, E.R. [Francis Bitter Magnet Lab., Cambridge, MA (United States)
1996-12-31
An experimental study was carried out on the tribological behavior of materials of interest in cryogenic applications, focusing on diamond and graphite. Both natural diamond (referred in the text as diamond) and chemical-vapor-deposition (CVD) diamond (CVD-diamond) were used. The experiment was carried out using a pin-on-disk tribometer capable of operating at cryogenic temperatures, from 4.2 to 293 K. Two basic scenarios of testing were used: (1) frictional coefficient ({mu}) vs velocity (v) characteristics at constant temperatures; (2) {mu} vs temperature (T) behavior at fixed sliding speeds. For diamond/CVD-diamond, graphite/CVD-diamond, stainless steel/CVD-diamond pairs, {mu}`s are virtually velocity independent. For each of diamond/graphite, alumina/graphite, and graphite/graphite pairs, the {partial_derivative}{mu}/{partial_derivative}v characteristic is favorable, i.e., positive. For diamond/CVD-diamond and graphite/CVD-diamond pairs, {mu}`s are nearly temperature independent between in the range 77 - 293 K. Each {mu} vs T plot for pin materials sliding on graphite disks has a peak at a temperature in the range 100 - 200 K.
Wills, A. S.; Zhitomirsky, M. E.; Canals, B.; Sanchez, J. P.; Bonville, P.; Dalmas de Réotier, P.; Yaouanc, A.
2006-01-01
Low-temperature powder neutron diffraction measurements are performed in the ordered magnetic state of the pyrochlore antiferromagnet Gd2Sn2O7. Symmetry analysis of the diffraction data indicates that this compound has the ground state predicted theoretically for a Heisenberg pyrochlore antiferromagnet with dipolar interactions. The difference in the magnetic structure of Gd2Sn2O7 andof nominally analogous Gd2Ti2O7 is found to be determined by a specific type of third-neighbour superexchange interaction on the pyrochlore lattice between spins across empty hexagons.
Dynamic rotor mode in antiferromagnetic nanoparticles
Lefmann, Kim; Jacobsen, H.; Garde, J.
2015-01-01
We present experimental, numerical, and theoretical evidence for an unusual mode of antiferromagnetic dynamics in nanoparticles. Elastic neutron scattering experiments on 8-nm particles of hematite display a loss of diffraction intensity with temperature, the intensity vanishing around 150 K...
Donnellan, Thomas; Maxwell, E A; Plumpton, C
1968-01-01
Lattice Theory presents an elementary account of a significant branch of contemporary mathematics concerning lattice theory. This book discusses the unusual features, which include the presentation and exploitation of partitions of a finite set. Organized into six chapters, this book begins with an overview of the concept of several topics, including sets in general, the relations and operations, the relation of equivalence, and the relation of congruence. This text then defines the relation of partial order and then partially ordered sets, including chains. Other chapters examine the properti
A synthetic diamond probe for low-energy X-ray dose measurements.
Assiamah, M; Nam, T L; Keddy, R J
2007-05-01
The desirable physical properties of diamond have made the mineral a choice material in radiation measurements. Diamond detectors are currently used extensively in high-energy physics. Their use for low-energy beams such as, for example, in mammography X-ray beams however, has not been fully investigated. This paper describes a diamond probe which has been constructed for the evaluation, as the radiation sensing material, of polycrystalline synthetic diamonds produced by chemical vapour deposition (CVD). The specimens were fabricated in wafer form and so the exposure orientation geometry of the diamond wafers, to give optimum absorption of the incident X-ray beam, was also investigated both experimentally and theoretically. The samples were characterized to obtain information regarding the elemental impurity levels, especially nitrogen, and consequently to establish the material quality. Nitrogen impurities and concentration levels in the diamond lattice have been shown to have a profound effect on the radiation detection properties of diamond. The probe described has the diamond surfaces metallized with titanium, platinum and gold to provide ohmic contacts. The probe was connected independently to both Wellhöfer Dosimetrie (model CU 500) and PTW Unidos E commercial electrometers. In all of the measurements, the incident radiation beam was normal to the edge of the diamond wafer to optimize absorption of the X-ray beam after establishing that this orientation was the optimum geometry. The results of the study are presented in both tabular and graphical forms.
Charge dynamics of the antiferromagnetically ordered Mott insulator
Han, Xing-Jie; Liu, Yu; Liu, Zhi-Yuan; Li, Xin; Chen, Jing; Liao, Hai-Jun; Xie, Zhi-Yuan; Normand, B.; Xiang, Tao
2016-10-01
We introduce a slave-fermion formulation in which to study the charge dynamics of the half-filled Hubbard model on the square lattice. In this description, the charge degrees of freedom are represented by fermionic holons and doublons and the Mott-insulating characteristics of the ground state are the consequence of holon-doublon bound-state formation. The bosonic spin degrees of freedom are described by the antiferromagnetic Heisenberg model, yielding long-ranged (Néel) magnetic order at zero temperature. Within this framework and in the self-consistent Born approximation, we perform systematic calculations of the average double occupancy, the electronic density of states, the spectral function and the optical conductivity. Qualitatively, our method reproduces the lower and upper Hubbard bands, the spectral-weight transfer into a coherent quasiparticle band at their lower edges and the renormalisation of the Mott gap, which is associated with holon-doublon binding, due to the interactions of both quasiparticle species with the magnons. The zeros of the Green function at the chemical potential give the Luttinger volume, the poles of the self-energy reflect the underlying quasiparticle dispersion with a spin-renormalised hopping parameter and the optical gap is directly related to the Mott gap. Quantitatively, the square-lattice Hubbard model is one of the best-characterised problems in correlated condensed matter and many numerical calculations, all with different strengths and weaknesses, exist with which to benchmark our approach. From the semi-quantitative accuracy of our results for all but the weakest interaction strengths, we conclude that a self-consistent treatment of the spin-fluctuation effects on the charge degrees of freedom captures all the essential physics of the antiferromagnetic Mott-Hubbard insulator. We remark in addition that an analytical approximation with these properties serves a vital function in developing a full understanding of the
Concepts for a low emittance-high capacity storage ring for the diamond light source
Bartolini, Riccardo; Evans, Gwyndaf; Sawhney, Kawal; Zegenhagen, Joerg
2017-01-01
The Diamond Light Source is investigating several paths for a possible machine upgrade to Diamond II. The exercise is driven by a joint assessment of the science capabilities opened by a very low emittance ring and the machine design that will underpin them. The consultation is made on a beamline-by-beamline basis and has highlighted a significant preference for lattices that combine both a low emittance and large capacity for IDs.
Diamond electronic properties and applications
Kania, Don R
1995-01-01
The use of diamond in electronic applications is not a new idea, but limitations in size and control of properties restricted the use of diamond to a few specialised applications. The vapour-phase synthesis of diamond, however, has facilitated serious interest in the development of diamond-based electronic devices. The process allows diamond films to be laid down over large areas. Both intrinsic and doped diamond films have a unique combination of extreme properties for high speed, high power and high temperature applications. The eleven chapters in Diamond: Electronic Properties and Applications, written by the world's foremost experts on the subject, give a complete characterisation of the material, in both intrinsic and doped forms, explain how to grow it for electronic applications, how to use the grown material, and a description of both passive and active devices in which it has been used with success. Diamond: Electronic Properties and Applications is a compendium of the available literature on the sub...
Gan, K K; Robichaud, A; Potenza, R; Kuleshov, S; Kagan, H; Kass, R; Wermes, N; Dulinski, W; Eremin, V; Smith, S; Sopko, B; Olivero, P; Gorisek, A; Chren, D; Kramberger, G; Schnetzer, S; Weilhammer, P; Martemyanov, A; Hugging, F; Pernegger, H; Lagomarsino, S; Manfredotti, C; Mishina, M; Trischuk, W; Dobos, D; Cindro, V; Belyaev, V; Duris, J; Claus, G; Wallny, R; Furgeri, A; Tuve, C; Goldstein, J; Sciortino, S; Sutera, C; Asner, D; Mikuz, M; Lo Giudice, A; Velthuis, J; Hits, D; Griesmayer, E; Oakham, G; Frais-Kolbl, H; Bellini, V; D'Alessandro, R; Cristinziani, M; Barbero, M; Schaffner, D; Costa, S; Goffe, M; La Rosa, A; Bruzzi, M; Schreiner, T; de Boer, W; Parrini, G; Roe, S; Randrianarivony, K; Dolenc, I; Moss, J; Brom, J M; Golubev, A; Mathes, M; Eusebi, R; Grigoriev, E; Tsung, J W; Mueller, S; Mandic, I; Stone, R; Menichelli, D
2011-01-01
With the commissioning of the LHC in 2010 and upgrades expected in 2015, ATLAS and CMS are planning to upgrade their innermost tracking layers with radiation hard technologies. Chemical Vapor Deposition diamond has been used extensively in beam conditions monitors as the innermost detectors in the highest radiation areas of BaBar, Belle, CDF and all LHC experiments. This material is now being considered as a sensor material for use very close to the interaction region where the most extreme radiation conditions exist Recently the RD42 collaboration constructed, irradiated and tested polycrystalline and single-crystal chemical vapor deposition diamond sensors to the highest fluences expected at the super-LHC. We present beam test results of chemical vapor deposition diamond up to fluences of 1.8 x 10(16) protons/cm(2) illustrating that both polycrystalline and single-crystal chemical vapor deposition diamonds follow a single damage curve. We also present beam test results of irradiated complete diamond pixel m...
Heteroepitaxial diamond growth
Markunas, R. J.; Rudder, R. A.; Posthill, J. B.; Thomas, R. E.; Hudson, G.
1994-02-01
Technical highlights from 1993 include the following: Growth Chemistries: A clear correlation was observed between ionization potential of feedstock gasses and critical power necessary for inductive coupling of the plasma and consequent diamond growth. Substrate preparation and epitaxial film quality: Ion-implantation of C and O has been coupled with either electrochemical etching or acid cleaning for surface preparation prior to homoepitaxial growth. Reactor modifications: Key improvements were made to the RF reactor to allow for long growths to consolidate substrates. Liquid mass flow controllers were added to precisely meter both the water and selected alcohol. Ion-implantation and lift off: Lift off of diamond platelets has been achieved with two processes. Ion-implantation of either C or O followed by annealing and implantation of either C or O followed by water based electrolysis. Diamond characterization: Development of novel detect characterization techniques: (1) Etch delineation of defects by exposure to propane torch flame. (2) Hydrogen plasma exposure to enhance secondary electron emission and provide non-topographical defect contrast. Acetylene will react at room temperature with sites created by partial desorption of oxygen from the (100) diamond surface. Thermal desorption measurements give an apparent activation energy for CO desorption from diamond (100) of 45 kcal/mol. Quantum chemical calculations indicate an activation energy of 38 kcal/mol for CO desorption. Ab initio calculations on (100) surfaces indicates that oxygen adsorbed at one dimer site has an effect on the dimerization of an adjacent site.
Structure and superconductivity of isotope-enriched boron-doped diamond
Evgeny A Ekimov, Vladimir A Sidorov, Andrey V Zoteev, Yury B Lebed, Joe D Thompson and Sergey M Stishov
2008-01-01
Full Text Available Superconducting boron-doped diamond samples were synthesized with isotopes of 10B, 11B, 13C and 12C. We claim the presence of a carbon isotope effect on the superconducting transition temperature, which supports the 'diamond-carbon'-related nature of superconductivity and the importance of the electron–phonon interaction as the mechanism of superconductivity in diamond. Isotope substitution permits us to relate almost all bands in the Raman spectra of heavily boron-doped diamond to the vibrations of carbon atoms. The 500 cm−1 Raman band shifts with either carbon or boron isotope substitution and may be associated with vibrations of paired or clustered boron. The absence of a superconducting transition (down to 1.6 K in diamonds synthesized in the Co–C–B system at 1900 K correlates with the small boron concentration deduced from lattice parameters.
Adhesion at WC/diamond interfaces - A theoretical study
Padmanabhan, Haricharan; Rao, M. S. Ramachandra; Nanda, B. R. K.
2015-06-01
We investigate the adhesion at the interface of face-centered tungsten-carbide (001) and diamond (001) from density-functional calculations. Four high-symmetry model interfaces, representing different lattice orientations for either side of the interface, are constructed to incorporate different degrees of strain arising due to lattice mismatch. The adhesion, estimated from the ideal work of separation, is found to be in the range of 4 - 7 J m-2 and is comparable to that of metal-carbide interfaces. Maximum adhesion occurs when WC and diamond slabs have the same orientation, even though such a growth induces large epitaxial strain at the interface. From electronic structure calculations, we attribute the adhesion to covalent interaction between carbon p-orbitals as well as partial ionic interaction between the tungsten d- and carbon p-orbitals across the interface.
Adhesion at WC/diamond interfaces - A theoretical study
Padmanabhan, Haricharan [Department of Engineering Design, Indian Institute of Technology Madras, Chennai – 600036 (India); Rao, M. S. Ramachandra [Department of Physics and Nano-Functional Materials Technology Centre, Indian Institute of Technology Madras, Chennai – 600036 (India); Nanda, B. R. K., E-mail: nandab@iitm.ac.in [Department of Physics, Indian Institute of Technology Madras, Chennai – 600036 (India)
2015-06-24
We investigate the adhesion at the interface of face-centered tungsten-carbide (001) and diamond (001) from density-functional calculations. Four high-symmetry model interfaces, representing different lattice orientations for either side of the interface, are constructed to incorporate different degrees of strain arising due to lattice mismatch. The adhesion, estimated from the ideal work of separation, is found to be in the range of 4 - 7 J m{sup −2} and is comparable to that of metal-carbide interfaces. Maximum adhesion occurs when WC and diamond slabs have the same orientation, even though such a growth induces large epitaxial strain at the interface. From electronic structure calculations, we attribute the adhesion to covalent interaction between carbon p-orbitals as well as partial ionic interaction between the tungsten d- and carbon p-orbitals across the interface.
Room Temperature Antiferromagnetic Ordering of Nanocrystalline Tb1.90Ni0.10O3
Mandal, J.; Dalal, M.; Sarkar, B. J.; Chakrabarti, P. K.
2017-02-01
Nanocrystalline Ni-doped terbium oxide (Tb1.90Ni0.10O3) has been synthesized by the co-precipitation method followed by annealing at 700°C for 6 h in vacuum. The crystallographic phase and the substitution of Ni2+ ions in the lattice of Tb2O3 are confirmed by Rietveld analysis of the x-ray diffraction pattern using the software MAUD. High-resolution transmission electron microscopy is also carried out to study the morphology of the sample. Magnetic measurements are carried out at different temperatures from 5 K to 300 K using a superconducting quantum interference device (SQUID) magnetometer. The dependence of the magnetization of Tb1.90Ni0.10O3 as a function of temperature ( M- T) and magnetic field ( M- H) suggests the presence of both paramagnetic and antiferromagnetic phase at room temperature, but antiferromagnetic phase dominates below ˜120 K. The lack of saturation in the M- H curve and good fitting of the M- T curve by the Johnston formula also indicate the presence of both paramagnetic and antiferromagnetic phase at room temperature. Interestingly, an antiferromagnetic to ferromagnetic phase transition is observed below ˜40 K. The result also shows a high value of magnetization at 5 K.
Large topological Hall effect in the non-collinear phase of an antiferromagnet.
Sürgers, Christoph; Fischer, Gerda; Winkel, Patrick; Löhneysen, Hilbert V
2014-03-05
Non-trivial spin arrangements in magnetic materials give rise to the topological Hall effect observed in compounds with a non-centrosymmetric cubic structure hosting a skyrmion lattice, in double-exchange ferromagnets and magnetically frustrated systems. The topological Hall effect has been proposed to appear also in presence of non-coplanar spin configurations and thus might occur in an antiferromagnetic material with a highly non-collinear and non-coplanar spin structure. Particularly interesting is a material where the non-collinearity develops not immediately at the onset of antiferromagnetic order but deep in the antiferromagnetic phase. This unusual situation arises in non-cubic antiferromagnetic Mn5Si3. Here we show that a large topological Hall effect develops well below the Néel temperature as soon as the spin arrangement changes from collinear to non-collinear with decreasing temperature. We further demonstrate that the effect is not observed when the material is turned ferromagnetic by carbon doping without changing its crystal structure.
Study of the effects of focused high-energy boron ion implantation in diamond
Ynsa, M. D.; Agulló-Rueda, F.; Gordillo, N.; Maira, A.; Moreno-Cerrada, D.; Ramos, M. A.
2017-08-01
Boron-doped diamond is a material with a great technological and industrial interest because of its exceptional chemical, physical and structural properties. At modest boron concentrations, insulating diamond becomes a p-type semiconductor and at higher concentrations a superconducting metal at low temperature. The most conventional preparation method used so far, has been the homogeneous incorporation of boron doping during the diamond synthesis carried out either with high-pressure sintering of crystals or by chemical vapour deposition (CVD) of films. With these methods, high boron concentration can be included without distorting significantly the diamond crystalline lattice. However, it is complicated to manufacture boron-doped microstructures. A promising alternative to produce such microstructures could be the implantation of focused high-energy boron ions, although boron fluences are limited by the damage produced in diamond. In this work, the effect of focused high-energy boron ion implantation in single crystals of diamond is studied under different irradiation fluences and conditions. Micro-Raman spectra of the sample were measured before and after annealing at 1000 °C as a function of irradiation fluence, for both superficial and buried boron implantation, to assess the changes in the diamond lattice by the creation of vacancies and defects and their degree of recovery after annealing.
Krstulic, J.F.
2000-01-27
The fundamental goal of this project was to develop additional capabilities to the diamond measuring prototype, work out technical difficulties associated with the original device, and perform automated measurements which are accurate and repeatable. For this project, FM and T was responsible for the overall system design, edge extraction, and defect extraction and identification. AccuGem provided a lab and computer equipment in Lawrence, 3D modeling, industry expertise, and sets of diamonds for testing. The system executive software which controls stone positioning, lighting, focusing, report generation, and data acquisition was written in Microsoft Visual Basic 6, while data analysis and modeling were compiled in C/C++ DLLs. All scanning parameters and extracted data are stored in a central database and available for automated analysis and reporting. The Phase 1 study showed that data can be extracted and measured from diamond scans, but most of the information had to be manually extracted. In this Phase 2 project, all data required for geometric modeling and defect identification were automatically extracted and passed to a 3D modeling module for analysis. Algorithms were developed which automatically adjusted both light levels and stone focus positioning for each diamond-under-test. After a diamond is analyzed and measurements are completed, a report is printed for the customer which shows carat weight, summarizes stone geometry information, lists defects and their size, displays a picture of the diamond, and shows a plot of defects on a top view drawing of the stone. Initial emphasis of defect extraction was on identification of feathers, pinpoints, and crystals. Defects were plotted color-coded by industry standards for inclusions (red), blemishes (green), and unknown defects (blue). Diamonds with a wide variety of cut quality, size, and number of defects were tested in the machine. Edge extraction, defect extraction, and modeling code were tested for
Competing antiferromagnetic and spin-glass phases in a hollandite structure
Crespo, Y.; Andreanov, A.; Seriani, N.
2013-07-01
We introduce a simple lattice model with Ising spins as a zeroth-order approximation of the hollandite-type magnetic compounds. We argue that geometrical frustration of the lattice in combination with nearest-neighbor antiferromagnetic (AFM) interactions are responsible for the appearance of a spin-glass phase in presence of disorder. We investigate this system numerically using parallel tempering. The model reproduces magnetic transitions present in some oxides with hollandite structure and displays a rich phenomenology: in the absence of disorder we have identified five different ground states, depending on the relative strength and sign of the interactions: one ferromagnetically ordered, three antiferromagnetically ordered, and one disordered, macroscopically degenerate ground state. Remarkably, for the sets of AFM couplings having an AFM ground state in the clean system, there exists a critical value of the disorder above which the ground state becomes a spin glass while maintaining all the couplings antiferromagnetically. This model presents this kind of transition with nearest-neighbor frustrated AFM interactions. We argue that this model is useful for understanding the relation between AFM coupling, disorder, and appearance of spin-glass phases.
Selli, Daniele; Baburin, Igor; Leoni, Stefano; Zhu, Zhen; Tománek, David; Seifert, Gotthard
2013-10-30
We investigate the interaction of a graphene monolayer with the C(111) diamond surface using ab initio density functional theory. To accommodate the lattice mismatch between graphene and diamond, the overlayer deforms into a wavy structure that binds strongly to the diamond substrate. The detached ridges of the wavy graphene overlayer behave electronically as free-standing polyacetylene chains with delocalized π electrons, separated by regions containing only sp(3) carbon atoms covalently bonded to the (111) diamond surface. We performed quantum transport calculations for different geometries of the system to study how the buckling of the graphene layer and the associated bonding to the diamond substrate affect the transport properties. The system displays high carrier mobility along the ridges and a wide transport gap in the direction normal to the ridges. These intriguing, strongly anisotropic transport properties qualify the hybrid graphene-diamond system as a viable candidate for electronic nanodevices.
Laser-excited photoemission spectroscopy study of superconducting boron-doped diamond
K. Ishizaka, R. Eguchi, S. Tsuda, T. Kiss, T. Shimojima, T. Yokoya, S. Shin, T. Togashi, S. Watanabe, C.-T. Chen, C.Q. Zhang, Y. Takano, M. Nagao, I. Sakaguchi, T. Takenouchi and H. Kawarada
2006-01-01
Full Text Available We have investigated the low-energy electronic state of boron-doped diamond thin film by the laser-excited photoemission spectroscopy. A clear Fermi-edge is observed for samples doped above the semiconductor–metal boundary, together with the characteristic structures at 150×n meV possibly due to the strong electron–lattice coupling effect. In addition, for the superconducting sample, we observed a shift of the leading edge below Tc indicative of a superconducting gap opening. We discuss the electron–lattice coupling and the superconductivity in doped diamond.
Mechanically induced degradation of diamond
Bouwelen, F V
1996-01-01
bombardment a mechanically induced graphitisation, as opposed to a thermally activated transformation, may occur locally on collision with the CVD diamond. Two types of diamond-graphite interfaces were observed: (111) planes of diamond parallel to the a-b planes of graphite and (111) planes of diamond, smoothly within the plane, connected to a-b planes of graphite. The thesis concludes with a summary of the results, conclusions and recommendations for further work. This thesis deals with the wear of diamond occurring during frictional sliding contact between diamonds. In the introduction, a literature survey on friction, wear and polishing behaviour of diamond, with some emphasis on the anisotropy, is presented and earlier work is discussed. A review of the existing theories is given, a new hypothesis is proposed and key-experiments for verification are identified. Electron microscopical techniques such as High Resolution Electron Microscopy (HREM) imaging and Electron Energy Loss Spectroscopy are described a...
Antiferromagnetic domain wall motion driven by spin-orbit torques
Shiino, Takayuki; Oh, Se-Hyeok; Haney, Paul M.; Lee, Seo-Won; Go, Gyungchoon; Park, Byong-Guk; Lee, Kyung-Jin
2016-01-01
We theoretically investigate dynamics of antiferromagnetic domain walls driven by spin-orbit torques in antiferromagnet/heavy metal bilayers. We show that spin-orbit torques drive antiferromagnetic domain walls much faster than ferromagnetic domain walls. As the domain wall velocity approaches the maximum spin-wave group velocity, the domain wall undergoes Lorentz contraction and emits spin-waves in the terahertz frequency range. The interplay between spin-orbit torques and the relativistic dynamics of antiferromagnetic domain walls leads to the efficient manipulation of antiferromagnetic spin textures and paves the way for the generation of high frequency signals from antiferromagnets. PMID:27588878
CVD diamond - fundamental phenomena
Yarbrough, W.A. [Pennsylvania State Univ., University Park (United States)
1993-01-01
This compilation of figures and diagrams addresses the basic physical processes involved in the chemical vapor deposition of diamond. Different methods of deposition are illustrated. For each method, observations are made of the prominent advantages and disadvantages of the technique. Chemical mechanisms of nucleation are introduced.
Biofunctionalization of diamond microelectrodes
Reitinger, Andreas Adam; Lud, Simon Quartus; Stutzmann, Martin; Garrido, Jose Antonio [Walter Schottky Institut, TU Muenchen (Germany); Hutter, Naima Aurelia; Richter, Gerhard; Jordan, Rainer [WACKER-Chair of Macromolecular Chemistry, TU Muenchen (Germany)
2010-07-01
In this work we present two main routes for the biofunctionalization of nanocrystalline diamond films, aiming at the application of diamond microelectrodes as amperometric biosensors. We report on direct covalent grafting of biomolecules on nanocrystalline diamond films via diazonium monophenyls and biphenyls as well as other linker molecules, forming self-assembled monolayers on the diamond surface. Monolayers with different functional head groups have been characterized. Patterning of the available functional groups using electron beam-induced chemical lithography allows the selective preparation of well-localized docking sites for the immobilization of biomolecules. Furthermore, polymer brushes are expected to enable novel paths for designing more advanced biosensing schemes, incorporating multifunctional groups and a higher loading capacity for biomolecules. Here, we focus on the preparation of polymer grafts by self-initiated photografting and photopolymerization. Further chemical modification of the grafted polymer brushes results in the introduction of additional functional molecules, paving the way for the incorporation of more complex molecular structures such as proteins. In a comparative study we investigate the advantages and disadvantages of both approaches.
Purely antiferromagnetic magnetoelectric random access memory
Kosub, Tobias; Kopte, Martin; Hühne, Ruben; Appel, Patrick; Shields, Brendan; Maletinsky, Patrick; Hübner, René; Liedke, Maciej Oskar; Fassbender, Jürgen; Schmidt, Oliver G.; Makarov, Denys
2017-01-01
Magnetic random access memory schemes employing magnetoelectric coupling to write binary information promise outstanding energy efficiency. We propose and demonstrate a purely antiferromagnetic magnetoelectric random access memory (AF-MERAM) that offers a remarkable 50-fold reduction of the writing threshold compared with ferromagnet-based counterparts, is robust against magnetic disturbances and exhibits no ferromagnetic hysteresis losses. Using the magnetoelectric antiferromagnet Cr2O3, we demonstrate reliable isothermal switching via gate voltage pulses and all-electric readout at room temperature. As no ferromagnetic component is present in the system, the writing magnetic field does not need to be pulsed for readout, allowing permanent magnets to be used. Based on our prototypes, we construct a comprehensive model of the magnetoelectric selection mechanisms in thin films of magnetoelectric antiferromagnets, revealing misfit induced ferrimagnetism as an important factor. Beyond memory applications, the AF-MERAM concept introduces a general all-electric interface for antiferromagnets and should find wide applicability in antiferromagnetic spintronics. PMID:28045029
Diamond growth in mantle fluids
Bureau, Hélène; Frost, Daniel J.; Bolfan-Casanova, Nathalie; Leroy, Clémence; Esteve, Imène; Cordier, Patrick
2016-11-01
In the upper mantle, diamonds can potentially grow from various forms of media (solid, gas, fluid) with a range of compositions (e.g. graphite, C-O-H fluids, silicate or carbonate melts). Inclusions trapped in diamonds are one of the few diagnostic tools that can constrain diamond growth conditions in the Earth's mantle. In this study, inclusion-bearing diamonds have been synthesized to understand the growth conditions of natural diamonds in the upper mantle. Diamonds containing syngenetic inclusions were synthesized in multi-anvil presses employing starting mixtures of carbonates, and silicate compositions in the presence of pure water and saline fluids (H2O-NaCl). Experiments were performed at conditions compatible with the Earth's geotherm (7 GPa, 1300-1400 °C). Results show that within the timescale of the experiments (6 to 30 h) diamond growth occurs if water and carbonates are present in the fluid phase. Water promotes faster diamond growth (up to 14 mm/year at 1400 °C, 7 GPa, 10 g/l NaCl), which is favorable to the inclusion trapping process. At 7 GPa, temperature and fluid composition are the main factors controlling diamond growth. In these experiments, diamonds grew in the presence of two fluids: an aqueous fluid and a hydrous silicate melt. The carbon source for diamond growth must be carbonate (CO32) dissolved in the melt or carbon dioxide species in the aqueous fluid (CO2aq). The presence of NaCl affects the growth kinetics but is not a prerequisite for inclusion-bearing diamond formation. The presence of small discrete or isolated volumes of water-rich fluids is necessary to grow inclusion-bearing peridotitic, eclogitic, fibrous, cloudy and coated diamonds, and may also be involved in the growth of ultradeep, ultrahigh-pressure metamorphic diamonds.
Brackett, Jeremy; Newman, Joseph; De Silva, Theja N.
2016-10-01
We study an effective fermion model on a square lattice to investigate the cooperation and competition of superconductivity and anti-ferromagnetism. In addition to particle tunneling and on-site interaction, a bosonic excitation mediated attractive interaction is also included in the model. We assume that the attractive interaction is mediated by spin fluctuations and excitations of Bose-Einstein condensation (BEC) in electronic systems and Bose-Fermi mixtures on optical lattices, respectively. Using an effective mean-field theory to treat both superconductivity and anti-ferromagnetism at equal footing, we study a single effective model relevant for both systems within the Landau energy functional approach and a linearized theory. Within our approaches, we find possible co-existence of superconductivity and anti-ferromagnetism for both electronic and cold-atomic models. Our linearized theory shows while spin fluctuations favor d-wave superconductivity and BEC excitations favor s-wave superconductivity.
Evidence for a gapped spin-liquid ground state in a kagome Heisenberg antiferromagnet.
Fu, Mingxuan; Imai, Takashi; Han, Tian-Heng; Lee, Young S
2015-11-06
The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of active debate. We conducted oxygen-17 single-crystal nuclear magnetic resonance (NMR) measurements of the spin-1/2 kagome lattice in herbertsmithite [ZnCu3(OH)6Cl2], which is known to exhibit a spinon continuum in the spin excitation spectrum. We demonstrated that the intrinsic local spin susceptibility χ(kagome), deduced from the oxygen-17 NMR frequency shift, asymptotes to zero below temperatures of 0.03J, where J ~ 200 kelvin is the copper-copper superexchange interaction. Combined with the magnetic field dependence of χ(kagome) that we observed at low temperatures, these results imply that the kagome Heisenberg antiferromagnet has a spin-liquid ground state with a finite gap.
Magnetostriction and Magnetostructural Domains in Antiferromagnetic YBa2Cu3O6.
Náfrádi, B; Keller, T; Hardy, F; Meingast, C; Erb, A; Keimer, B
2016-01-29
We use high-resolution neutron Larmor diffraction and capacitative dilatometry to investigate spontaneous and forced magnetostriction in undoped, antiferromagnetic YBa_{2}Cu_{3}O_{6.0}, the parent compound of a prominent family of high-temperature superconductors. Upon cooling below the Néel temperature T_{N}=420 K, Larmor diffraction reveals the formation of magnetostructural domains of characteristic size ∼240 nm. In the antiferromagnetic state, dilatometry reveals a minute (4×10^{-6}) orthorhombic distortion of the crystal lattice in external magnetic fields. We attribute these observations to exchange striction and spin-orbit coupling induced magnetostriction, respectively, and show that they have an important influence on the thermal and charge transport properties of undoped and lightly doped cuprates.
P. Sahebsara
2006-09-01
Full Text Available The self-energy-functional approach is a powerful many-body tool to investigate different broken symmetry phases of strongly correlated electron systems. We use the variational cluster perturbation theory (also called the variational cluster approximation to investigate the interplay between the antiferromagnetism and d-wave superconductivity of κ-(ET2 X conductors. These compounds are described by the so-called dimer Hubbard model, with various values of the on-site repulsion U and diagonal hopping amplitude t. At strong coupling, our zero-temperature calculations show a transition from Néel antiferromagnetism to a spin-liquid phase with no long range order, at around t ~ 0.9. At lower values of U, we find d-wave superconductivity. Taking into account the point group symmetries of the lattice, we find a transition between dx2-y2 and dxy pairing symmetries, the latter happening for smaller values of U.
DMRG studies of the frustrated kagome antiferromagnets and the application to volborthite
Gong, Shou-Shu; Sheng, D. N.; Yang, Kun
Motivated by the recent magnetization measurements on the high-quality single crystals of the kagome antiferromagnet volborthite, we study the ground state and magnetization properties of two kagome models proposed from the electronic structure simulations, which treat the volborthite as either the coupled trimers or the coupled frustrated chains on the kagome lattice. We study the models using density-matrix renormalization group on the cylinder geometry with the system width up to 4 legs. We find a quantum phase diagram of the models with changing couplings, and identify the magnetic properties of each phase. In the antiferromagnetic phases, we also study the magnetization curve and the different phases in the magnetic field. Finally, we compare the magetization properties of the models with the experimental observations of volborthite. NSF DMR-1157490, DMR-1408560, and the State of Florida.
Weak antiferromagnetic order and superconductivity in UPt 3 studied by neutron scattering
van Dijk, N. H.; Rodière, P.; Fåk, B.; Huxley, A.; Flouquet, J.
2002-07-01
The heavy-fermion superconductor UPt 3 is one of the best-studied examples of systems that show unconventional superconductivity. Below a transition temperature of Tc=0.55 K a complex phase diagram with three different superconducting phases is observed as a function of temperature, magnetic field, and pressure. The weak antiferromagnetic order ( TN=6 K) with an ordered moment of only 0.02 μB/U atom is believed to play a crucial role in the existence of multiple superconducting phases, as it can act as a symmetry-breaking field for the vector order parameter of the unconventional superconductivity. We review recent progress in neutron scattering measurements on the weak antiferromagnetic order as a function of magnetic field, pressure, and Pd doping and on the superconducting flux-line lattice. The relation between the magnetic and superconducting properties is discussed.
Forty years of development in diamond tools
The growth of the diamond industry in Western Countries since the First World War is surveyed. The articles described deal specifically with the development of the industrial diamond and diamond tool sector in different countries. All data point to continuing rapid expansion in the diamond tool sector. The West consumes 80 percent of world industrial diamond production. Diamond consumption increased sharply in the U.S. during World War 2. There are 300 diamond manufacturers in the U.S. today. In 1940, there were 25. In Japan, consumption of industrial diamonds has increased several times. In Italy, there has been a 75 fold increase in the production of diamond tools since 1959.
Potts Model on Maple Leaf Lattice with Pure Three-Site Interaction
WANG Zhou-Fei; CHEN Li
2005-01-01
We use Monte Carlo method to study three-state Potts model on maple leaf lattice with pure three-site interaction. The critical behavior of both ferromagnetic and antiferromagnetic cases is studied. Our results confirm that the critical behavior of the ferromagnetic model is independent of the lattice details and lies in the universality class of the three-state ferromagnetic Potts model. For the antiferromagnetic case the transition is of the first order. We have calculated the energy jump and critical temperature in this area. We find there is a tricritical point separating the first order and second order phases for this system.
Schaefer, Stefan [DESY (Germany). Neumann Inst. for Computing
2016-11-01
These configurations are currently in use in many on-going projects carried out by researchers throughout Europe. In particular this data will serve as an essential input into the computation of the coupling constant of QCD, where some of the simulations are still on-going. But also projects computing the masses of hadrons and investigating their structure are underway as well as activities in the physics of heavy quarks. As this initial project of gauge field generation has been successful, it is worthwhile to extend the currently available ensembles with further points in parameter space. These will allow to further study and control systematic effects like the ones introduced by the finite volume, the non-physical quark masses and the finite lattice spacing. In particular certain compromises have still been made in the region where pion masses and lattice spacing are both small. This is because physical pion masses require larger lattices to keep the effects of the finite volume under control. At light pion masses, a precise control of the continuum extrapolation is therefore difficult, but certainly a main goal of future simulations. To reach this goal, algorithmic developments as well as faster hardware will be needed.
Paramagnetic and Antiferromagnetic Spin Seebeck Effect
Wu, Stephen
We report on the observation of the longitudinal spin Seebeck effect in both antiferromagnetic and paramagnetic insulators. By using a microscale on-chip local heater, it is possible to generate a large thermal gradient confined to the chip surface without a large increase in the total sample temperature. This technique allows us to easily access low temperatures (200 mK) and high magnetic fields (14 T) through conventional dilution refrigeration and superconducting magnet setups. By exploring this regime, we detect the spin Seebeck effect through the spin-flop transition in antiferromagnetic MnF2 when a large magnetic field (>9 T) is applied along the easy axis direction. Using the same technique, we are also able to resolve a spin Seebeck effect from the paramagnetic phase of geometrically frustrated antiferromagnet Gd3Ga5O12 (gadolinium gallium garnet) and antiferromagnetic DyScO3 (DSO). Since these measurements occur above the ordering temperatures of these two materials, short-range magnetic order is implicated as the cause of the spin Seebeck effect in these systems. The discovery of the spin Seebeck effect in these two materials classes suggest that both antiferromagnetic spin waves and spin excitations from short range magnetic order may be used to generate spin current from insulators and that the spin wave spectra of individual materials are highly important to the specifics of the longitudinal spin Seebeck effect. Since insulating antiferromagnets and paramagnets are far more common than the typical insulating ferrimagnetic materials used in spin Seebeck experiments, this discovery opens up a large new class of materials for use in spin caloritronic devices. All authors acknowledge support of the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division. The use of facilities at the Center for Nanoscale Materials, was supported by the U.S. DOE, BES under Contract No. DE-AC02-06CH11357.
Frustrated Magnetism in Low-Dimensional Lattices
Tovar, Mayra
2011-12-01
In this dissertation we present the results of a theoretical investigation of spin models on two-dimensional and quasi one-dimensional lattices, all unified under the concept of quantum frustrated antiferromagnetism, and all discussing various aspects of the antiferromagnetic Heisenberg model on the kagome lattice. In the Introduction (Chapter 1), we discuss at some length such concepts as frustration and superexchange, among others, which are of common relevance in the rest of the chapters. In Chapter 2, we study the effect of Dzyaloshinskii-Moriya (DM) interactions on the zero-temperature magnetic susceptibility of systems whose low energy can be described by short-range valence bond states. Our work shows that this treatment is consistent with the experimentally observed non-vanishing susceptibility---in the specified temperature limit---of the spin-1/2 kagome antiferromagnetic compound ZnCu3(OH)6Cl2, also known as herbertsmithite. Although the objective of this work is explaining the aforementioned characteristic of the experimental system, our methods are more general and we apply them to the checkerboard and Shastry-Sutherland lattices as well. In Chapter 3, we discuss our findings in the study of ghost-mediated domain wall interactions in the diamondback ladder. These domain walls are the the spin excitations---the kinks and the antikinks---separating the ground states along one chain of the ladder. While as individual entities an antikink is energy costly and a kink energy free, our study finds that both interact via the ghosts that they produce in the opposite side of the ladder from where they are located. Through the study of these ghosts, we find that domain walls proliferate in the system above a critical value of the system's coupling constants. It is this proliferation that makes their treatment as free, non-interacting particles impossible, so we study here their interactions both quantitatively and qualitatively, in a region where the latter are
Spin-wave multiple excitations in nanoscale classical Heisenberg antiferromagnets
Hou, Zhuofei [University of Georgia, Athens; Landau, David P [University of Georgia, Athens; Stocks, George Malcolm [ORNL; Brown, G. [Florida State University, Tallahassee
2015-02-17
Monte Carlo and spin dynamics techniques have been used to perform large-scale simulations of the dynamic behavior of a nanoscale, classical, Heisenberg antiferromagnet on a simple-cubic lattice with linear sizes L≤ 40 at a temperature below the Neel temperature. In this study, nanoparticles are modeled with completely free boundary conditions, i.e., six free surfaces, and nanofilms are modeled with two free surfaces in the spatial z direction and periodic boundaries parallel to the surfaces in the xy direction, which are compared to the infinite system with periodic boundary conditions. The temporal evolutions of spin configurations were determined numerically from coupled equations of motion for individual spins using a fast spin dynamics algorithm with the fourth-order Suzuki-Trotter decomposition of exponential operators, with initial spin configurations generated by Monte Carlo simulations. The local dynamic structure factor S(q,ω) was calculated from the local space- and time-displaced spin-spin correlation function. Multiple excitation peaks for wave vectors within the first Brillouin zone appear in the spin-wave spectra of the transverse component of dynamic structure factor S^{T} (q,ω) in the nanoscale classical Heisenberg antiferromagnet, which are lacking if periodic boundary conditions are used. With the assumption of q-space spin-wave reflections with broken momentum conservation due to free-surface confinements, we successfully explained those spectra quantitatively in the linear dispersion region. Meanwhile, we also observed two unexpected quantized spin-wave excitation modes in the spatial z direction in nanofilms for S^{T} (q,ω) not expected in bulk systems. In conclusion, the results of this study indicate the presence of unexpected forms of spin-wave excitation behavior that have yet to be observed experimentally but could be directly tested through neutron scattering experiments on nanoscale RbMnF_{3} particles or
Astronomers debate diamonds in space
1999-04-01
diamonds --a million times smaller than a millimetre and thus called "nanodiamonds"-- from a sample of the Orgueil meteorite, and then subjected them to infrared spectroscopy. The researchers conclude that nanodiamonds of a certain kind, defective ones in which some atoms of the lattice are missing, have a "chemical signature" that matches the one detected in the stars very closely. Footnote on ISO ESA's infrared space telescope, ISO, was put into orbit in November 1995, by an Ariane 44P launcher from the European Spaceport in Kourou, French Guiana. Its operational phase lasted till 16 May, 1998, almost a year longer than expected. As an unprecedented observatory for infrared astronomy, able to examine cool and hidden places in the Universe, ISO made nearly 30 000 scientific observations. These are now available to the scientific community via the ISO Archive (http://www.iso.vilspa.esa.es) at the ISO Data Centre, in Villafranca, near Madrid, Spain.
Lattice effects on Laughlin wave functions and parent Hamiltonians
Glasser, Ivan; Cirac, J. Ignacio; Sierra, Germán; Nielsen, Anne E. B.
2016-12-01
We investigate lattice effects on wave functions that are lattice analogs of bosonic and fermionic Laughlin wave functions with number of particles per flux ν =1 /q in the Landau levels. These wave functions are defined analytically on lattices with μ particles per lattice site, where μ may be different than ν . We give numerical evidence that these states have the same topological properties as the corresponding continuum Laughlin states for different values of q and for different fillings μ . These states define, in particular, particle-hole symmetric lattice fractional quantum Hall states when the lattice is half filled. On the square lattice it is observed that for q ≤4 this particle-hole symmetric state displays the topological properties of the continuum Laughlin state at filling fraction ν =1 /q , while for larger q there is a transition towards long-range ordered antiferromagnets. This effect does not persist if the lattice is deformed from a square to a triangular lattice, or on the kagome lattice, in which case the topological properties of the state are recovered. We then show that changing the number of particles while keeping the expression of these wave functions identical gives rise to edge states that have the same correlations in the bulk as the reference lattice Laughlin states but a different density at the edge. We derive an exact parent Hamiltonian for which all these edge states are ground states with different number of particles. In addition this Hamiltonian admits the reference lattice Laughlin state as its unique ground state of filling factor 1 /q . Parent Hamiltonians are also derived for the lattice Laughlin states at other fillings of the lattice, when μ ≤1 /q or μ ≥1 -1 /q and when q =4 also at half filling.
Structure and properties of diamond and diamond-like films
Clausing, R.E. [Oak Ridge National Lab., TN (United States)
1993-01-01
This section is broken into four parts: (1) introduction, (2) natural IIa diamond, (3) importance of structure and composition, and (4) control of structure and properties. Conclusions of this discussion are that properties of chemical vapor deposited diamond films can compare favorably with natural diamond, that properties are anisotropic and are a strong function of structure and crystal perfection, that crystal perfection and morphology are functions of growth conditions and can be controlled, and that the manipulation of texture and thereby surface morphology and internal crystal perfection is an important step in optimizing chemically deposited diamond films for applications.
Genetics Home Reference: Diamond-Blackfan anemia
... Home Health Conditions Diamond-Blackfan anemia Diamond-Blackfan anemia Printable PDF Open All Close All Enable Javascript ... view the expand/collapse boxes. Description Diamond-Blackfan anemia is a disorder of the bone marrow . The ...
Nanocrystalline diamond films for biomedical applications
Pennisi, Cristian Pablo; Alcaide, Maria
2014-01-01
Nanocrystalline diamond films, which comprise the so called nanocrystalline diamond (NCD) and ultrananocrystalline diamond (UNCD), represent a class of biomaterials possessing outstanding mechanical, tribological, and electrical properties, which include high surface smoothness, high corrosion re...
Biological applications of nanocrystalline diamond
Williams, Oliver; Daenen, Michael; Haenen, Ken
2007-01-01
Nanocrystalline diamond films have generated substantial interest in recent years due to their low cost, extreme properties and wide application arena. Diamond is chemically inert, has a wide electrochemical window and is stable in numerous harsh environments. Nanocrystalline diamond has the advantage of being readily grown on a variety of substrates at very low thickness, resulting in smooth conformal coatings with high transparency. These films can be doped from highly insulating to metalli...
Yang Yukun; Han Tao
1995-01-01
@@ The geologic condition of Shengli Oilfield (SLOF)is complicated and the range of the rock drillability is wide. For more than 20 years,Shengli Drilling Technology Research Institute, in view of the formation conditions of SLOF,has done a lot of effort and obtained many achivements in design,manufacturing technology and field service. Up to now ,the institute has developed several ten kinds of diamond bits applicable for drilling and coring in formations from extremely soft to hard.
Blackley, W.S.; Scattergood, R.O.
1988-12-01
A new research initiative will be undertaken to investigate the critical cutting depth concepts for single point diamond turning of brittle, amorphous materials. Inorganic glasses and a brittle, thermoset polymer (organic glass) are the principal candidate materials. Interrupted cutting tests similar to those done in earlier research are Ge and Si crystals will be made to obtain critical depth values as a function of machining parameters. The results will provide systematic data with which to assess machining performance on glasses and amorphous materials
Long-range interactions in lattice field theory
Rabin, J.M.
1981-06-01
Lattice quantum field theories containing fermions can be formulated in a chirally invariant way provided long-range interactions are introduced. It is established that in weak-coupling perturbation theory such a lattice theory is renormalizable when the corresponding continuum theory is, and that the continuum theory is indeed recovered in the perturbative continuum limit. In the strong-coupling limit of these theories one is led to study an effective Hamiltonian describing a Heisenberg antiferromagnet with long-range interactions. Block-spin renormalization group methods are used to find a critical rate of falloff of the interactions, approximately as inverse distance squared, which separates a nearest-neighbor-antiferromagnetic phase from a phase displaying identifiable long-range effects. A duality-type symmetry is present in some block-spin calculations.
Magnetic remanent states in antiferromagnetically coupled multilayers
Kiselev, N.S., E-mail: m.kyselov@ifw-dresden.d [IFW Dresden, Postfach 270116, D-01171 Dresden (Germany); Donetsk Institute for Physics and Technology, 83114 Donetsk (Ukraine); Roessler, U.K.; Bogdanov, A.N. [IFW Dresden, Postfach 270116, D-01171 Dresden (Germany); Hellwig, O. [San Jose Research Center, Hitachi Global Storage Technologies, San Jose, CA 95135 (United States)
2010-05-15
In antiferromagnetically coupled multilayers with perpendicular anisotropy unusual multidomain textures can be stabilized due to a close competition between long-range demagnetization fields and short-range interlayer exchange coupling. In particular, the formation and evolution of specific topologically stable planar defects within the antiferromagnetic ground state, i.e. wall-like structures with a ferromagnetic configuration extended over a finite width, explain configurational hysteresis phenomena recently observed in [Co/Pt(Pd)]/Ru and [Co/Pt]/NiO multilayers. Within a phenomenological theory, we have analytically derived the equilibrium sizes of these 'ferroband' defects as functions of the antiferromagnetic exchange, a bias magnetic field, and geometrical parameters of the multilayers. In the magnetic phase diagram, the existence region of the ferrobands mediates between the regions of patterns with sharp antiferromagnetic domain walls and regular arrays of ferromagnetic stripes. The theoretical results are supported by magnetic force microscopy images of the remanent states observed in [Co/Pt]/Ru.
Direct measurement of antiferromagnetic domain fluctuations.
Shpyrko, O. G.; Isaacs, E. D.; Logan, J. M.; Feng, Y.; Aeppli, G.; Jaramillo, R.; Kim, H. C.; Rosenbaum, T. F.; Zschack, P.; Sprung, M.; Narayanan, S.; Sandy, A.; Univ. of Chicago; Univ. College London
2007-05-03
Measurements of magnetic noise emanating from ferromagnets owing to domain motion were first carried out nearly 100 years ago1, and have underpinned much science and technology2, 3. Antiferromagnets, which carry no net external magnetic dipole moment, yet have a periodic arrangement of the electron spins extending over macroscopic distances, should also display magnetic noise. However, this must be sampled at spatial wavelengths of the order of several interatomic spacings, rather than the macroscopic scales characteristic of ferromagnets. Here we present a direct measurement of the fluctuations in the nanometer-scale superstructure of spin- and charge-density waves associated with antiferromagnetism in elemental chromium. The technique used is X-ray photon correlation spectroscopy, where coherent X-ray diffraction produces a speckle pattern that serves as a 'fingerprint' of a particular magnetic domain configuration. The temporal evolution of the patterns corresponds to domain walls advancing and retreating over micrometer distances. This work demonstrates a useful measurement tool for antiferromagnetic domain wall engineering, but also reveals a fundamental finding about spin dynamics in the simplest antiferromagnet: although the domain wall motion is thermally activated at temperatures above 100 K, it is not so at lower temperatures, and indeed has a rate that saturates at a finite value--consistent with quantum fluctuations--on cooling below 40 K.
Antiferromagnetism in chromium alloy single crystals
Bjerrum Møller, Hans; Trego, A.L.; Mackintosh, A.R.
1965-01-01
The antiferromagnetism of single crystals of dilute alloys of V, Mn and Re in Cr has been studied at 95°K and 300°K by neutron diffraction. The addition of V causes the diffraction peaks to decrease in intensity and move away from (100), while Mn and Re cause them to increase and approach (100) so...
Superconductivity in CVD diamond films.
Takano, Yoshihiko
2009-06-24
A beautiful jewel of diamond is insulator. However, boron doping can induce semiconductive, metallic and superconducting properties in diamond. When the boron concentration is tuned over 3 × 10(20) cm(-3), diamonds enter the metallic region and show superconductivity at low temperatures. The metal-insulator transition and superconductivity are analyzed using ARPES, XAS, NMR, IXS, transport and magnetic measurements and so on. This review elucidates the physical properties and mechanism of diamond superconductor as a special superconductivity that occurs in semiconductors.
Antiferromagnet-long-period structure phase transition in RMn2O5 oxides
Men'shenin, V. V.; Nikolaev, V. V.; Dmitriev, A. V.
2011-07-01
An analysis of the magnetic phase transition from an antiferromagnetic into an incommensurate phase in oxides RMn2O5 has been performed. It has been shown that this is a second-order phase transition and that it can occur through one of complete irreducible representations of the space group Pbam, i.e., without a decrease in the symmetry of the crystal lattice. It has been established that the decrease in the electric polarization of the oxides in this transition is due to the development of long-period magnetic ordering.
Orbital degeneracy removed by charge order in triangular antiferromagnet AgNiO2
Wawrzynska, E.; Coldea, R.; Wheeler, E M; Mazin, I. I.; Johannes, M. D.; Sorgel, T.; Jansen, M; Ibberson, R. M.; Radaelli, P. G.
2007-01-01
We report a high-resolution neutron diffraction study on the orbitally-degenerate spin-1/2 hexagonal antiferromagnet AgNiO2. A structural transition to a tripled unit cell with expanded and contracted NiO6 octahedra indicates root(3) x root(3) charge order on the Ni triangular lattice. This suggests charge order as a possible mechanism of lifting the orbital degeneracy in the presence of charge fluctuations, as an alternative to Jahn-Teller distortions. A novel magnetic ground state is observ...
Wawrzynska, E.; Coldea, R.; Wheeler, E M; Sorgel, T.; Jansen, M; Ibberson, R. M.; Radaelli, P. G.; Koza, M. M.
2007-01-01
We report a high-resolution neutron diffraction study of the crystal and magnetic structure of the orbitally-degenerate frustrated metallic magnet AgNiO2. At high temperatures the structure is hexagonal with a single crystallographic Ni site, low-spin Ni3+ with spin-1/2 and two-fold orbital degeneracy, arranged in an antiferromagnetic triangular lattice with frustrated spin and orbital order. A structural transition occurs upon cooling below 365 K to a tripled hexagonal unit cell containing t...
Néel temperature of quasi-low-dimensional Heisenberg antiferromagnets.
Yasuda, C; Todo, S; Hukushima, K; Alet, F; Keller, M; Troyer, M; Takayama, H
2005-06-03
The Néel temperature T(N) of quasi-one- and quasi-two-dimensional antiferromagnetic Heisenberg models on a cubic lattice is calculated by Monte Carlo simulations as a function of interchain (interlayer) to intrachain (intralayer) coupling J(')/J down to J(')/J approximately = 10(-3). We find that T(N) obeys a modified random-phase approximationlike relation for small J(')/J with an effective universal renormalized coordination number, independent of the size of the spin. Empirical formulas describing T(N) for a wide range of J(') and useful for the analysis of experimental measurements are presented.
Gammelmark, Søren; Eckardt, André
2013-01-01
We theoretically study the adiabatic preparation of an antiferromagnetic phase in a mixed Mott insulator of two bosonic atom species in a one-dimensional optical lattice. In such a system one can engineer a tunable parabolic inhomogeneity by controlling the difference of the trapping potentials f...... that during the preparation finite size effects will play a crucial role for a system of realistic size. The experiment that we propose can be realized, for example, using atomic mixtures of rubidium 87 with potassium 41, or ytterbium 168 with ytterbium 174....
Quantum phase transitions in the Heisenberg J1-J2 triangular antiferromagnet in a magnetic field
Ye, Mengxing; Chubukov, Andrey V.
2017-01-01
We present the zero-temperature phase diagram of a Heisenberg antiferromagnet on a frustrated triangular lattice with nearest-neighbor (J1) and next-nearest-neighbor (J2) interactions, in a magnetic field. We show that the classical model has an accidental degeneracy for all J2/J1 and all fields, but the degeneracy is lifted by quantum fluctuations. We show that at large spin S , for J2/J11 , the transition remains first order, with a finite hysteresis width, but for S =1 /2 and, possibly, S =1 , there appears a new intermediate phase without a quasiclassical long-range order.
Emergent Power-Law Phase in the 2D Heisenberg Windmill Antiferromagnet: A Computational Experiment.
Jeevanesan, Bhilahari; Chandra, Premala; Coleman, Piers; Orth, Peter P
2015-10-23
In an extensive computational experiment, we test Polyakov's conjecture that under certain circumstances an isotropic Heisenberg model can develop algebraic spin correlations. We demonstrate the emergence of a multispin U(1) order parameter in a Heisenberg antiferromagnet on interpenetrating honeycomb and triangular lattices. The correlations of this relative phase angle are observed to decay algebraically at intermediate temperatures in an extended critical phase. Using finite-size scaling we show that both phase transitions are of the Berezinskii-Kosterlitz-Thouless type, and at lower temperatures we find long-range Z(6) order.
Spin transport of the frustrated quasi-two-dimensional XY-like antiferromagnet
Lima, L. S.
2017-01-01
We use the Self Consistent Harmonic Approximation together with the Kubo formalism of the Linear Response Theory to study the spin transport in the two-dimensional frustrated Heisenberg antiferromagnet in a square lattice with easy-plane ion single anisotropy. The regular part of the spin conductivity σreg(ω) is determined for several values of the critical ion single parameter Dc, that separates the low D region from the large D quantum paramagnetic phase. We have obtained an abrupt change in the spin conductivity in the discontinuity points of the graphic Dc vs. η, where the system presents a quantum phase transition.
Large off-diagonal magnetoelectric coupling in the quantum paraelectric antiferromagnet EuTiO3
Shvartsman, V. V.; Borisov, P.; Kleemann, W.; Kamba, S.; Katsufuji, T.
2010-02-01
The third-order E2H2 -type magnetoelectric (ME) response of polycrystalline EuTiO3 changes sign under magnetic bias and shows a large anomaly at the antiferromagnetic (AF)-paramagnetic phase boundary below TN≈5.3K . It is attributed to critical fluctuations of the AF order parameter reinforced by quantum paraelectric polar correlations. The underlying biquadratic spin-lattice coupling involves electric field induced Dzyaloshinskii-Moriya interaction as described within mean-field approximation. Single domaining by ME annealing (or cooling) significantly enhances the response by additional EH and EH2 effects.
Macroscopic anisotropy and symmetry breaking in the pyrochlore antiferromagnet Gd2Ti2O7
Hassan, A. K.; Lévy, L. P.; Darie, C.; Strobel, P.
2003-06-01
In the Heisenberg antiferromagnet Gd2Ti2O7, the exchange interactions are geometrically frustrated by the pyrochlore lattice structure. This ESR study reveals a strong temperature dependent anisotropy with respect to a [111] body diagonal below a temperature TA=80 K, despite the spin only nature of the Gd3+ ion. Anisotropy and symmetry breaking can nevertheless appear through the superexchange interaction. In the presence of anisotropic exchanges, short range planar correlations restricted to specific Kagomé planes are sufficient to explain the two ESR modes studied in this work.
Unusual finite size effects on critical temperature in fcc Ising antiferromagnets
Pommier, J.; Diep, H. T.; Ghazali, A.; Lallemand, P.
1988-04-01
A new multispin coding technique is presented for Monte Carlo simulation of antiferromagnetic Ising spin systems on an fcc lattice. The nearest- and next-nearest-neighbor interactions J1 and J2 are included. This technique allows a considerable gain in CPU time and computer memory. As a first application, we have studied samples of 4L3 spins with L up to 48. An unusual behavior of the critical temperature with increasing L is found in the case of nearest-neighbor interaction in zero field. Finite size effects on the locations of tricrical points in the (T,J2/J1) plane are discussed.
Dual Lattice of ℤ-module Lattice
Futa Yuichi
2017-07-01
Full Text Available In this article, we formalize in Mizar [5] the definition of dual lattice and their properties. We formally prove that a set of all dual vectors in a rational lattice has the construction of a lattice. We show that a dual basis can be calculated by elements of an inverse of the Gram Matrix. We also formalize a summation of inner products and their properties. Lattice of ℤ-module is necessary for lattice problems, LLL(Lenstra, Lenstra and Lovász base reduction algorithm and cryptographic systems with lattice [20], [10] and [19].
Optimized resonating valence bond state in square lattice: correlations & excitations
Z Nourbakhsh
2009-09-01
Full Text Available We consider RVB state as a variational estimate for the ground state of Heisenberg antiferromagnet in square lattice. We present numerical calculation of energy, spin-spin correlation function and spin excitation spectrum. We show, that the quantum flactuations reduce of magnetization respect to Neel order. Our results are in good agreement with other methods such as spin-wave calculation and series expansions.
Diamond Pixel Detectors and 3D Diamond Devices
Venturi, N.
2016-12-01
Results from detectors of poly-crystalline chemical vapour deposited (pCVD) diamond are presented. These include the first analysis of data of the ATLAS Diamond Beam Monitor (DBM). The DBM module consists of pCVD diamond sensors instrumented with pixellated FE-I4 front-end electronics. Six diamond telescopes, each with three modules, are placed symmetrically around the ATLAS interaction point. The DBM tracking capabilities allow it to discriminate between particles coming from the interaction point and background particles passing through the ATLAS detector. Also, analysis of test beam data of pCVD DBM modules are presented. A new low threshold tuning algorithm based on noise occupancy was developed which increases the DBM module signal to noise ratio significantly. Finally first results from prototypes of a novel detector using pCVD diamond and resistive electrodes in the bulk, forming a 3D diamond device, are discussed. 3D devices based on pCVD diamond were successfully tested with test beams at CERN. The measured charge is compared to that of a strip detector mounted on the same pCVD diamond showing that the 3D device collects significantly more charge than the planar device.
Possible form of multi-polar interaction in cubic lattice
Sakai, Osamu; Shiina, Ryousuke; Shiba, Hiroyuki
2003-05-01
The invariant form of interaction between multi-poles, including the octupole, is studied for the simple cubic (SC), body centered and face centered cubic lattices. The coupling terms can be arranged in a way similar to that of the hopping matrix between the LCAO's. A table for SC by Shiina et al. (J. Phys. Soc. Japan 66 (1997) 1741) is generalized for the general wave number case of the three types of lattice. Recent experimental result of TmTe is thereby analyzed. The development of the ferromagnetic moment below the anti-ferromagnetic transition under the anti-ferro quadrupolar order phase is discussed in this connection.
Spin Waves in 2D ferromagnetic square lattice stripe
Ahmed, Maher Z.
2011-01-01
In this work, the area and edges spin wave calculations were carried out using the Heisenberg Hamiltonian and the tridiagonal method for the 2D ferromagnetic square lattice stripe, where the SW modes are characterized by a 1D in-plane wave vector $q_x$. The results show a general and an unexpected feature that the area and edge spin waves only exist as optic modes. This behavior is also seen in 2D Heisenberg antiferromagnetic square lattice. This absence of the acoustic modes in the 2D square...
Possible form of multi-polar interaction in cubic lattice
Sakai, Osamu; Shiina, Ryousuke; Shiba, Hiroyuki
2003-05-01
The invariant form of interaction between multi-poles, including the octupole, is studied for the simple cubic (SC), body centered and face centered cubic lattices. The coupling terms can be arranged in a way similar to that of the hopping matrix between the LCAO's. A table for SC by Shiina et al. (J. Phys. Soc. Japan 66 (1997) 1741) is generalized for the general wave number case of the three types of lattice. Recent experimental result of TmTe is thereby analyzed. The development of the ferromagnetic moment below the anti-ferromagnetic transition under the anti-ferro quadrupolar order phase is discussed in this connection.
New statistical lattice model with double honeycomb symmetry
Naji, S.; Belhaj, A.; Labrim, H.; Bhihi, M.; Benyoussef, A.; El Kenz, A.
2014-04-01
Inspired from the connection between Lie symmetries and two-dimensional materials, we propose a new statistical lattice model based on a double hexagonal structure appearing in the G2 symmetry. We first construct an Ising-1/2 model, with spin values σ = ±1, exhibiting such a symmetry. The corresponding ground state shows the ferromagnetic, the antiferromagnetic, the partial ferrimagnetic and the topological ferrimagnetic phases depending on the exchange couplings. Then, we examine the phase diagrams and the magnetization using the mean field approximation (MFA). Among others, it has been suggested that the present model could be localized between systems involving the triangular and the single hexagonal lattice geometries.
The stability of a crystal with diamond structure for patchy particles with tetrahedral symmetry.
Noya, Eva G; Vega, Carlos; Doye, Jonathan P K; Louis, Ard A
2010-06-21
The phase diagram of model anisotropic particles with four attractive patches in a tetrahedral arrangement has been computed at two different values of the range of the potential, with the aim of investigating the conditions under which a diamond crystal can be formed. We find that the diamond phase is never stable for our longer-ranged potential. At low temperatures and pressures, the fluid freezes into a body-centered-cubic solid that can be viewed as two interpenetrating diamond lattices with a weak interaction between the two sublattices. Upon compression, an orientationally ordered face-centered-cubic crystal becomes more stable than the body-centered-cubic crystal, and at higher temperatures, a plastic face-centered-cubic phase is stabilized by the increased entropy due to orientational disorder. A similar phase diagram is found for the shorter-ranged potential, but at low temperatures and pressures, we also find a region over which the diamond phase is thermodynamically favored over the body-centered-cubic phase. The higher vibrational entropy of the diamond structure with respect to the body-centered-cubic solid explains why it is stable even though the enthalpy of the latter phase is lower. Some preliminary studies on the growth of the diamond structure starting from a crystal seed were performed. Even though the diamond phase is never thermodynamically stable for the longer-ranged model, direct coexistence simulations of the interface between the fluid and the body-centered-cubic crystal and between the fluid and the diamond crystal show that at sufficiently low pressures, it is quite probable that in both cases the solid grows into a diamond crystal, albeit involving some defects. These results highlight the importance of kinetic effects in the formation of diamond crystals in systems of patchy particles.
Understanding the source: The nitrogen isotope composition of Type II mantle diamonds
Mikhail, Sami; Howell, Dan; Jones, Adrian; Milledge, Judith; Verchovsky, Sasha
2010-05-01
Diamonds can be broadly subdivided into 2 groups based on their nitrogen content; type I with > 10ppm nitrogen and type II with growth nitrogen can be incorporated into diamond as a compatible element in a closed system and therefore the N/C ratio in the source can be depleted by Rayleigh fractionation as the first diamonds to crystallise will partition nitrogen atoms into their lattice as a 1:1 substitution for carbon atoms (type I diamonds). However nitrogen may behave as an incompatible element in diamond (and be a compatible element in the metasomatic fluid), this coupled with an open system would lead to the removal of nitrogen by the metasomatic fluids, thus causing the source to progressively become depleted in nitrogen. Continued diamond crystallization in either system will produce diamonds with ever decreasing nitrogen concentrations with time, possibly to the point of them being almost nitrogen free. 2- It is conceivable that type I & II diamonds found in the same deposit and sharing a common paragenesis (eclogitic or peridotitic) may have formed from different metasomatic fluids in separate diamond forming events. The latter has been proposed for samples from the Cullinan mine (South Africa) based on their carbon isotope compositions (3). Both models can be tested using the stable isotope compositions of carbon and nitrogen with the N/C ratio of the diamonds in a given population with varying nitrogen content (from type I to type II). 1.D. G. Pearson, D. Canil, S. B. Shirey, D. H. Heinrich, K. T. Karl, in Treatise on Geochemistry. (Pergamon, Oxford, 2003), pp. 171-275. 2.C. McCammon, Science 293, 813 (August 3, 2001, 2001). 3.A. E. Moore, South African Journal of Geology 112, 23 (March 1, 2009, 2009).
Spin-lattice coupling in iron jarosite
Buurma, A.J.C.; Handayani, I.P. [Zernike Institute for Advanced Materials, University of Groningen, Nijenborgh 4, 9747 AG Groningen (Netherlands); Mufti, N. [Max Planck Institute for Chemical Physics of Solids, Noethnitzer Str. 40, 01187 Dresden (Germany); Blake, G.R.; Loosdrecht, P.H.M. van [Zernike Institute for Advanced Materials, University of Groningen, Nijenborgh 4, 9747 AG Groningen (Netherlands); Palstra, T.T.M., E-mail: t.t.m.palstra@rug.nl [Zernike Institute for Advanced Materials, University of Groningen, Nijenborgh 4, 9747 AG Groningen (Netherlands)
2012-11-15
We have studied the magnetoelectric coupling of the frustrated triangular antiferromagnet iron jarosite using Raman spectroscopy, dielectric measurements and specific heat. Temperature dependent capacitance measurements show an anomaly in the dielectric constant at T{sub N}. Specific heat data indicate the presence of a low frequency Einstein mode at low temperature. Raman spectroscopy confirms the presence of a new mode below T{sub N} that can be attributed to folding of the Brillouin zone. This mode shifts and sharpens below T{sub N}. We evaluate the strength of the magnetoelectric coupling using the symmetry unrestricted biquadratic magnetoelectric terms in the free energy. - Graphical abstract: Sketch of two connected triangles formed by Fe{sup 3+} spins (red arrows) in the hexagonal basal plane of potassium iron jarosite. An applied magnetic field (H) below the antiferromagnetic ordering temperature induces shifts of the hydroxy ligands, giving rise to local electrical dipole moments (blue arrows). These electric displacements cancel out in pairwise fashion by symmetry. Ligand shifts are confined to the plane and shown by shadowing. Highlights: Black-Right-Pointing-Pointer Evidence has been found for spin-lattice coupling in iron jarosite. Black-Right-Pointing-Pointer A new optical Raman mode appears below T{sub N} and shifts with temperature. Black-Right-Pointing-Pointer The magnetodielectric coupling is mediated by superexchange. Black-Right-Pointing-Pointer Symmetry of Kagome magnetic lattice causes local electrical dipole moments to cancel.
Dynamic zero modes of Dirac fermions and competing singlet phases of antiferromagnetic order
Goswami, Pallab; Si, Qimiao
2017-06-01
In quantum spin systems, singlet phases often develop in the vicinity of an antiferromagnetic order. Typical settings for such problems arise when itinerant fermions are also present. In this paper, we develop a theoretical framework for addressing such competing orders in an itinerant system, described by Dirac fermions strongly coupled to an O(3) nonlinear sigma model. We focus on two spatial dimensions, where upon disordering the antiferromagnetic order by quantum fluctuations the singular tunneling events also known as (anti)hedgehogs can nucleate competing singlet orders in the paramagnetic phase. In the presence of an isolated hedgehog configuration of the nonlinear sigma model field, we show that the fermion determinant vanishes as the dynamic Euclidean Dirac operator supports fermion zero modes of definite chirality. This provides a topological mechanism for suppressing the tunneling events. Using the methodology of quantum chromodynamics, we evaluate the fermion determinant in the close proximity of magnetic quantum phase transition, when the antiferromagnetic order-parameter field can be described by a dilute gas of hedgehogs and antihedgehogs. We show how the precise nature of emergent singlet order is determined by the overlap between dynamic fermion zero modes of opposite chirality, localized on the hedgehogs and antihedgehogs. For a Kondo-Heisenberg model on the honeycomb lattice, we demonstrate the competition between spin Peierls order and Kondo singlet formation, thereby elucidating its global phase diagram. We also discuss other physical problems that can be addressed within this general framework.
Relief of frustration in the Heisenberg pyrochlore antiferromagnet Gd2Pt2O7
Hallas, A. M.; Sharma, A. Z.; Cai, Y.; Munsie, T. J.; Wilson, M. N.; Tachibana, M.; Wiebe, C. R.; Luke, G. M.
2016-10-01
The gadolinium pyrochlores Gd2B2O7 are among the best realizations of antiferromagnetically coupled Heisenberg spins on a pyrochlore lattice. We present a magnetic characterization of Gd2Pt2O7 , a unique member of this family. Magnetic susceptibility, heat capacity, and muon spin relaxation measurements show that Gd2Pt2O7 undergoes an antiferromagnetic ordering transition at TN=1.6 K. This transition is strongly first order, as indicated by the sharpness of the heat capacity anomaly, thermal hysteresis in the magnetic susceptibility, and a nondivergent relaxation rate in μ SR . The form of the heat capacity below TN suggests that the ground state is an anisotropic collinear antiferromagnet with an excitation spectrum that is gapped by 0.245(1) meV. The ordering temperature in Gd2Pt2O7,TN=1.6 K, is a substantial 160% increase from other gadolinium pyrochlores, which are all known to order at 1 K or lower. We attribute this enhancement in TN to the B -site cation, platinum. Despite being nonmagnetic, platinum has a filled 5 d t2 g orbital and an empty 5 d eg orbital that can facilitate superexchange. Thus, the magnetic frustration in Gd2Pt2O7 is partially "relieved," thereby promoting magnetic order.
Superfluid and antiferromagnetic phases in ultracold fermionic quantum gases
Gottwald, Tobias
2010-08-27
In this thesis several models are treated, which are relevant for ultracold fermionic quantum gases loaded onto optical lattices. In particular, imbalanced superfluid Fermi mixtures, which are considered as the best way to realize Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) states experimentally, and antiferromagnetic states, whose experimental realization is one of the next major goals, are examined analytically and numerically with the use of appropriate versions of the Hubbard model. The usual Bardeen-Cooper-Schrieffer (BCS) superconductor is known to break down in a magnetic field with a strength exceeding the size of the superfluid gap. A spatially inhomogeneous spin-imbalanced superconductor with a complex order parameter known as FFLO-state is predicted to occur in translationally invariant systems. Since in ultracold quantum gases the experimental setups have a limited size and a trapping potential, we analyze the realistic situation of a non-translationally invariant finite sized Hubbard model for this purpose. We first argue analytically, why the order parameter should be real in a system with continuous coordinates, and map our statements onto the Hubbard model with discrete coordinates defined on a lattice. The relevant Hubbard model is then treated numerically within mean field theory. We show that the numerical results agree with our analytically derived statements and we simulate various experimentally relevant systems in this thesis. Analogous calculations are presented for the situation at repulsive interaction strength where the N'eel state is expected to be realized experimentally in the near future. We map our analytical results obtained for the attractive model onto corresponding results for the repulsive model. We obtain a spatially invariant unit vector defining the direction of the order parameter as a consequence of the trapping potential, which is affirmed by our mean field numerical results for the repulsive case. Furthermore, we observe
N. A. Poklonski; N. M. Lapchuk; A. V. Khomich; LU Fan-Xiu; TANG Wei-Zhong; V. G. Ralchenko; I. I. Vlasov; M. V. Chukichev; Sambuu Munkhtsetseg
2007-01-01
Electron spin resonance (ESR) in polycrystalline diamond films grown by dc arc-jet and microwave plasma chemical vapour deposition is studied. The films with nitrogen impurity concentration up to 8 × 1018 cm-3 are also characterized by Raman, cathodoluminescence and optical absorption spectra. The ESR signal from P1 centre with g-factor of 2.0024 (nitrogen impurity atom occupying C site in diamond lattice) is found to exhibit an inversion with increasing the microwave power in an H102 resonator. The spin inversion effect could be of interest for further consideration of N-doped diamonds as a medium for masers operated at room temperature.
High efficiency diamond solar cells
Gruen, Dieter M.
2008-05-06
A photovoltaic device and method of making same. A layer of p-doped microcrystalline diamond is deposited on a layer of n-doped ultrananocrystalline diamond such as by providing a substrate in a chamber, providing a first atmosphere containing about 1% by volume CH.sub.4 and about 99% by volume H.sub.2 with dopant quantities of a boron compound, subjecting the atmosphere to microwave energy to deposit a p-doped microcrystalline diamond layer on the substrate, providing a second atmosphere of about 1% by volume CH.sub.4 and about 89% by volume Ar and about 10% by volume N.sub.2, subjecting the second atmosphere to microwave energy to deposit a n-doped ultrananocrystalline diamond layer on the p-doped microcrystalline diamond layer. Electrodes and leads are added to conduct electrical energy when the layers are irradiated.
Designing of concrete diamond sawblade
ZHANG Shao-he; DING Xin-yu; ZHOU Jia-xiang
2005-01-01
By analyzing the abrasive theory of concrete diamond sawblade, the proposal that the diamond should be selected by its function in cutting concrete is presented. The part of the big grit diamonds cut rock, and the part of the small grit diamonds improve the wearability of the matrix. The contrast tests are done with different shapes of sawbaldes in split segment, slant "U" slot segment, sandwich segment, turbo segment and three-slot segment. The special shapes of sawblades can improve the effect of cooling and the removing ability of the rock powder. The data of tests show that the efficiency of cutting and the life of sawblades are improved by designing the diamond prescription and using the especial geometry of segment.
Murtazaev, A. K.; Babaev, A. B.; Ataeva, G. Ya.
2017-01-01
The thermodynamic properties and phase transitions in a two-dimensional strongly diluted threevertex antiferromagnetic Potts model on a triangular lattice have been investigated using the Monte Carlo method. The systems with linear dimensions of L × L = N, where L = 18-48, have been considered. It has been shown using the method of fourth-order Binder cumulants that, upon the introduction of nonmagnetic impurities into the spin system described by the two-dimensional antiferromagnetic Potts model, the firstorder phase transition changes to a second-order phase transition.
Insight into the antiferromagnetic structure manipulated by electronic reconstruction
Cui, B.; Li, F.; Song, C.; Peng, J. J.; Saleem, M. S.; Gu, Y. D.; Li, S. N.; Wang, K. L.; Pan, F.
2016-10-01
Antiferromagnetic (AFM) materials, with robust rigidity to magnetic field perturbations and ultrafast spin dynamics, show great advantages in information storage and have developed into a fast-emerging field of AFM spintronics. However, a direct characterization of spin alignments in AFM films has been challenging, and their manipulation by lattice distortion and magnetic proximity is inevitably accompanied by "ferromagnetic" features within the AFM matrix. Here we resolve the G -type AFM structure of SrCo O2.5 and find that the interfacial AFM structure could be modulated intrinsically from in plane to out of plane with a canted angle of 60∘ by the charge transfer and orbital reconstruction in SrCo O2.5/L a2 /3S r1 /3Mn O3 heterostructures both experimentally and theoretically. Such an interfacial AFM reconfiguration caused by electronic reconstruction does not cause the ferromagnetic feature and changes the magnetization switching process of L a2 /3S r1 /3Mn O3 from in plane to perpendicular to the plane, in turn. Our study not only reveals the coupling between charge, orbital, and AFM structure, but also provides a unique approach to manipulating AFM structure.
Ultrafast Band Engineering and Transient Spin Currents in Antiferromagnetic Oxides.
Gu, Mingqiang; Rondinelli, James M
2016-04-29
We report a dynamic structure and band engineering strategy with experimental protocols to induce indirect-to-direct band gap transitions and coherently oscillating pure spin-currents in three-dimensional antiferromagnets (AFM) using selective phononic excitations. In the Mott insulator LaTiO3, we show that a photo-induced nonequilibrium phonon mode amplitude destroys the spin and orbitally degenerate ground state, reduces the band gap by 160 meV and renormalizes the carrier masses. The time scale of this process is a few hundreds of femtoseconds. Then in the hole-doped correlated metallic titanate, we show how pure spin-currents can be achieved to yield spin-polarizations exceeding those observed in classic semiconductors. Last, we demonstrate the generality of the approach by applying it to the non-orbitally degenerate AFM CaMnO3. These results advance our understanding of electron-lattice interactions in structures out-of-equilibrium and establish a rational framework for designing dynamic phases that may be exploited in ultrafast optoelectronic and optospintronic devices.
Spin-dynamics simulations of the triangular antiferromagnetic XY model*
Nho, Kwangsik; Landau, D. P.
2003-03-01
Using Monte Carlo and spin-dynamics methods, we have studied the dynamic behavior of the classical, antiferromagnetic XY model on a triangular lattice. The temporal evolutions of spin configurations were obtained by solving numerically the coupled equations of motion for each spin using fourth-order Suzuki-Trotter decompositions of exponential operators. We calculated the dynamic structure factor S(q,w) for momentum q and frequency w. Below T_KT (Kosteritz-Thouless transition), both the in-plane (S^xx) and out-of-plane (S^zz) components exhibit very strong and sharp spin-wave peaks. Well above T_KT, S^xx and S^zz apparently display a central peak, and spin-wave signatures are still seen in S^zz. In addition, we also observed an almost dispersionless domain-wall peak at high w below Tc (Ising transition), where long-range order appears in the staggered chirality[1]. We found that our results demonstrate the consistency of the dynamic finite-size scaling theory for the characteristic frequency wm and S(q,w). *Supported by NSF [1] D.H. Lee, J.D. Joannopoulos, J.W. Negele, and D.P. Landau, Phys. Rev. Lett. 52, 433 (1984)
Spin-dynamics simulations of the antiferromagnetic triangular XY model*
Nho, Kwangsik; Landau, D. P.
2002-03-01
Using Monte Carlo and spin-dynamics methods, we have simulated the dynamic behavior of the classical, antiferromagnetic XY model on a triangular lattice. The temporal evolutions of spin configurations were obtained by solving numerically the coupled equations of motion for each spin using fourth-order Suzuki-Trotter decompositions of exponential operators. From space-and time-displaced spin-spin correlation functions and their space-time Fourier transforms we obtained the dynamic structure factor S(q,w) for momentum q and frequency w. Below T_c, where long-range order appears in the staggered chirality[1], S(q,w) exhibits very strong and sharp spin-wave peaks in the in-plane-component S^xx. We also observe two-spin-wave peaks at low w and an almost dispersionless domain-wall peak at high w. Above T_c, a weak spin-wave peak persists but the domain-wall peak disappears for all q. We have calculated the dispersion relation and the linewidth of the spin-wave peak in S^xx by fitting the line shape to simple Lorentzians. *Supported by NSF [1] D.H. Lee, J.D. Joannopoulos, J.W. Negele, and D.P. Landau, Phys. Rev. Lett. 52, 433 (1984)
Three-dimensional antiferromagnetic CP(N-1) models.
Delfino, Francesco; Pelissetto, Andrea; Vicari, Ettore
2015-05-01
We investigate the critical behavior of three-dimensional antiferromagnetic CP(N-1) (ACP(N-1)) models in cubic lattices, which are characterized by a global U(N) symmetry and a local U(1) gauge symmetry. Assuming that critical fluctuations are associated with a staggered gauge-invariant (Hermitian traceless matrix) order parameter, we determine the corresponding Landau-Ginzburg-Wilson (LGW) model. For N=3 this mapping allows us to conclude that the three-component ACP(2) model undergoes a continuous transition that belongs to the O(8) vector universality class, with an effective enlargement of the symmetry at the critical point. This prediction is confirmed by numerical analyses of the finite-size scaling behaviors of the ACP(2) and the O(8) vector models, which show the same universal features at their transitions. We also present a renormalization-group (RG) analysis of the LGW theories for N≥4. We compute perturbative series in two different renormalization schemes and analyze the corresponding RG flow. We do not find stable fixed points that can be associated with continuous transitions.
Piermarini, Gasper J.
It has often been said that scientific advances are made either in a dramatic and revolutionary way, or, as in the case of the diamond anvil cell (DAC), in a slow and evolutionary manner over a period of several years. For more than 2 decades, commencing in 1958, the DAC developed stepwise from a rather crude qualitative instrument to the sophisticated quantitative research tool it is today, capable of routinely producing sustained static pressures in the multi-megabar range and readily adaptable to numerous scientific measurement techniques because of its optical accessibility, miniature size, and portability.
Ozima, M.; Zashu, S.
1983-03-01
He-3/He-4 isotopic ratio analyses of 13 diamond stones from unspecified mines in South Africa yield values ranging from less than 10 to the -7th to 0.00032 + or - 0.000025. The latter value is higher than the primordial He-3/He-4 ratio in meteorites, and close to the ratio for solar type He. It is suggested that these elevated values may represent primitive He which has evolved little, in view of its minute increase in radiogenic He-4, since the earth's formation.
Heteroepitaxial Diamond Growth
1993-01-12
interstitials, respectively. The energies required for the planar to puckered distortion are 4.3 eV on Ni(l 11), 3.0 eV with the Na interstitial, 3.6 eV with H...give consideration to the crystallographic I alignment between diamond tiles to minimize dislocation densities at the " seams ". 3 Methods of checking the...crystallographic alignment (non-destructively) and assessing the dislocation densities at seams must be used to establish the viability of 3 any
许斌; 李木森; 尹龙卫; 崔建军; 宫建红
2003-01-01
The metallic film surrounding a diamond single crystal, which plays an important role in the diamond growth from an Fe-Ni-C system, has been successfully investigated by using transmission-electron microscopy (TEM),Raman spectroscopy and x-ray photo-electron spectroscopy (XPS). Diamond and graphite were not found in surface layer (near diamond) of the film by TEM and Raman spectroscopy, but a parallel relationship exists between the (111) plane of γ-(Fe,Ni) and the (100) plane of (Fe, Ni)3C in this region. Compared with that of solvent metal (catalyst) near diamond, the binding energy in the valence bands of iron, nickel and carbon atoms of the film has an increase of 0.9 eV. According to the microstructures on the film obtained by the TEM, Raman spectra, and XPS, the catalytic mechanism of the film may be assumed as follows. In the surface layer of the film,iron and nickel atoms in the γ-(Fe, Ni) lattice can absorb carbon atoms in the (Fe, Ni)3C lattice and make them transform to an sp3-like state. Then carbon atoms with the sp3-like structure are separated from the (Fe,Ni)3C and stack on the growing diamond crystal. This study provides a direct evidence for the diamond growth from a metallic catalyst-graphite system under high temperature and high pressure.
Inducing spin-dependent tunneling to probe magnetic correlations in optical lattices
Pedersen, Kim-Georg; Andersen, Brian; Syljuåsen, Olav;
2012-01-01
We suggest a simple experimental method for probing antiferromagnetic spin correlations of two-component Fermi gases in optical lattices. The method relies on a spin selective Raman transition to excite atoms of one spin species to their first excited vibrational mode where the tunneling is large...
Monte Carlo study of the double and super-exchange model with lattice distortion
Suarez, J R; Vallejo, E; Navarro, O [Instituto de Investigaciones en Materiales, Universidad Nacional Autonoma de Mexico, Apartado Postal 70-360, 04510 Mexico D. F. (Mexico); Avignon, M, E-mail: jrsuarez@iim.unam.m [Institut Neel, Centre National de la Recherche Scientifique (CNRS) and Universite Joseph Fourier, BP 166, 38042 Grenoble Cedex 9 (France)
2009-05-01
In this work a magneto-elastic phase transition was obtained in a linear chain due to the interplay between magnetism and lattice distortion in a double and super-exchange model. It is considered a linear chain consisting of localized classical spins interacting with itinerant electrons. Due to the double exchange interaction, localized spins tend to align ferromagnetically. This ferromagnetic tendency is expected to be frustrated by anti-ferromagnetic super-exchange interactions between neighbor localized spins. Additionally, lattice parameter is allowed to have small changes, which contributes harmonically to the energy of the system. Phase diagram is obtained as a function of the electron density and the super-exchange interaction using a Monte Carlo minimization. At low super-exchange interaction energy phase transition between electron-full ferromagnetic distorted and electron-empty anti-ferromagnetic undistorted phases occurs. In this case all electrons and lattice distortions were found within the ferromagnetic domain. For high super-exchange interaction energy, phase transition between two site distorted periodic arrangement of independent magnetic polarons ordered anti-ferromagnetically and the electron-empty anti-ferromagnetic undistorted phase was found. For this high interaction energy, Wigner crystallization, lattice distortion and charge distribution inside two-site polarons were obtained.
Macroscopic Quantum Coherence in Antiferromagnetic Molecular Magnets
HU Hui; LO Rong; ZHU Jia-Lin; XIONG Jia-Jiong
2001-01-01
The macroscopic quantum coherence in a biaxial antiferromagnetic molecular magnet in the presence of magnetic field acting parallel to its hard anisotropy axis is studied within the two-sublattice model. On the basis of instanton technique in the spin-coherent-state path-integral representation, both the rigorous Wentzel-Kramers-Brillouin exponent and pre-exponential factor for the ground-state tunnel splitting are obtained. We find that the quantum fluctuations around the classical paths can not only induce a new quantum phase previously reported by Chiolero and Loss (Phys. Rev. Lett. 80 (1998) 169), but also have great influence on the intensity of the ground-state tunnel splitting. Those features clearly have no analogue in the ferromagnetic molecular magnets. We suggest that they may be the universal behaviors in all antiferromagnetic molecular magnets. The analytical results are complemented by exact diagonalization calculation.
Macroscopic Quantum Coherence in Antiferromagnetic Molecular Magnets
HUHui; LURong; 等
2001-01-01
The macroscopic quantum coherence in a biaxial antiferromagnetic molecular magnet in the presence of magnetic field acting parallel to its hard anisotropy axis is studied within the two-sublattice model.On the basis of instanton technique in the spin-coherent-state path-integral representation,both the rigorous Wentzel-Kramers-Brillouin exponent and pre-exponential factor for the ground-state tunnel splitting are obtained.We find that the quantum fluctuations around the classical paths can not only induce a new quantum phase previously reported by Chiolero and Loss (Phys.Rev.Lett.80(1998)169),but also have great influence on the intensity of the ground-state tunnel splitting.Those features clearly have no analogue in the ferromagnetic molecular magnets.We suggest that they may be the universal behaviors in all antiferromagnetic molecular magnets.The analytical results are complemented by exact diagonalization calculation.
Shape-induced anisotropy in antiferromagnetic nanoparticles
H. Gomonay; Kondovych, S.; Loktev, V.
2013-01-01
High fraction of the surface atoms considerably enhances the influence of size and shape on the magnetic and electronic properties of nanoparticles. Shape effects in ferromagnetic nanoparticles are well understood and allow to set and control the parameters of a sample that affect its magnetic anisotropy during production. In the present paper we study the shape effects in the other widely used magnetic materials -- antiferromagnets, -- which possess vanishingly small or zero macroscopic magn...
Spin-Mechanical Inertia in Antiferromagnet
2016-01-01
The conservation of angular momentum has served as a guiding principle in the coupled dynamics of quantum spins and mechanical rotations. However, in an antiferromagnet with vanishing magnetization, new fundamental rules are required to properly describe spin-mechanical phenomena. Here we demonstrate that the Neel order dynamics affects the mechanical motion of a rigid body by modifying its inertia tensor in the presence of strong magnetocrystalline anisotropy. This effect depends on temperat...
Spin Transport in Ferromagnetic and Antiferromagnetic Textures
Akosa, Collins A.
2016-12-07
In this dissertation, we provide an accurate description of spin transport in magnetic textures and in particular, we investigate in detail, the nature of spin torque and magnetic damping in such systems. Indeed, as will be further discussed in this thesis, the current-driven velocity of magnetic textures is related to the ratio between the so-called non-adiabatic torque and magnetic damping. Uncovering the physics underlying these phenomena can lead to the optimal design of magnetic systems with improved efficiency. We identified three interesting classes of systems which have attracted enormous research interest (i) Magnetic textures in systems with broken inversion symmetry: We investigate the nature of magnetic damping in non-centrosymmetric ferromagnets. Based on phenomenological and microscopic derivations, we show that the magnetic damping becomes chiral, i.e. depends on the chirality of the magnetic texture. (ii) Ferromagnetic domain walls, skyrmions and vortices: We address the physics of spin transport in sharp disordered magnetic domain walls and vortex cores. We demonstrate that upon spin-independent scattering, the non-adiabatic torque can be significantly enhanced. Such an enhancement is large for vortex cores compared to transverse domain walls. We also show that the topological spin currents owing in these structures dramatically enhances the non-adiabaticity, an effect unique to non-trivial topological textures (iii) Antiferromagnetic skyrmions: We extend this study to antiferromagnetic skyrmions and show that such an enhanced topological torque also exist in these systems. Even more interestingly, while such a non-adiabatic torque inuences the undesirable transverse velocity of ferromagnetic skyrmions, in antiferromagnetic skyrmions, the topological non-adiabatic torque directly determines the longitudinal velocity. As a consequence, scaling down the antiferromagnetic skyrmion results in a much more efficient spin torque.
Synthesis of Diamond Films with Pulsed Plasma
1992-03-01
Diamond and Diamond-Like Films, The Electrochemical Society , Los Angeles, California, Volume 89-12, 114, May 1989. M. Aklufi and D. Brock, "Synthesis Of...Diamond Films By Microwave Generated Pulsed Plasmas," Proceedings of The Second International Symposium On Diamond Materials, The Electrochemical Society , Washington, DC, Volume 91-8, ’ 39, May 1991.
Multipartite Entanglement of a Tetrahedron Lattice
ZHANG Rong; ZHU Shi-Qun; HAO Xiang
2006-01-01
Three-dimensional Heiscnberg model in the form of a tetrahedron lattice is investigated. The concurrence and multipartite entanglement are calculated through 2-concurrence C and 4-concurrence C4. The concurrence C and multipartite entanglement C4 depend on different coupling strengths Ji and are decreased when the temperature T is increased. For a symmetric tetraledron lattice, the concurrence C is symmetric about J1 when J2 is negative while the multipartite entanglement C4 is symmetric about J1 wlen J2 ＜ 2. For a regular tetrahedron lattice, the concurrence C of ground state is 1/3 for ferromagnetic case while C=0 for antiferromagnetic case. However, there is no multipartite entanglement since C4=0 in a regular tetraledron lattice. The external magnetic field B can increase the maximum value of the concurrence CB and induce two or three peaks in CB. There is a peak in the multipartite entanglement C4B when C4B is varied as a function of the temperature T. This peak is mainly induced by the magnetic field B.
Extreme Mechanics of Probing the Ultimate Strength of Nanotwinned Diamond
Li, Bing; Sun, Hong; Chen, Changfeng
2016-09-01
Recently synthesized nanotwinned diamond (NTD) exhibits unprecedented Vickers hardness exceeding 200 GPa [Q. Huang et al., Nature (London) 510, 250 (2014)]. This extraordinary finding challenges the prevailing understanding of material deformation and stress response under extreme loading conditions. Here we unveil by first-principles calculations a novel indenter-deformation generated stress confinement mechanism that suppresses the graphitization or bond collapse failure modes commonly known in strong covalent solids, leading to greatly enhanced peak stress and strain range in the indented diamond lattice. Moreover, the twin boundaries in NTD promote a strong stress concentration that drives preferential bond realignments, producing a giant indentation strain stiffening. These results explain the exceptional indentation strength of NTD and offer insights into the extreme mechanics of the intricate interplay of the indenter and indented crystal in probing ultrahard materials.
Interlaced particle systems and tilings of the Aztec diamond
Fleming, Benjamin J
2010-01-01
Motivated by the problem of domino tilings of the Aztec diamond, a weighted particle system is defined on $N$ lines, with line $j$ containing $j$ particles. The particles are restricted to lattice points from 0 to $N$, and particles on successive lines are subject to an interlacing constraint. It is shown that marginal distributions for this particle system can be computed exactly. This in turn is used to give unified derivations of a number of fundamental properties of the tiling problem, for example the evaluation of the number of distinct configurations and the relation to the GUE minor process. An interlaced particle system associated with the domino tiling of a certain half Aztec diamond is similarly defined and analyzed.
Spin transfer in antiferromagnets (Conference Presentation)
Moriyama, Takahiro
2016-10-01
Since antiferromagnets (AFMs) have no spontaneous magnetization unlike ferromagnetic materials, it is not easy to manipulate the magnetic moments in AFMs by external magnetic field. However, recent theoretical studies suggest that it is possible to manipulate the magnetization in AFMs by spin-transfer-torque in a similar manner to ferromagnetic materials. In this study, we perform spin-toque ferromagnetic resonance (ST-FMR) measurements on FeNi/NiO/Pt multilayers to experimentally investigate the interaction between the spin current and the magnetic moments of antiferromagnetic NiO. The spin current is injected to the NiO by the spin Hall effect in Pt. The monotonous change in the FMR linewidth of this system with respect to the spin current can be interpreted in a way that the spin current is transferred through the NiO and interacts with the FeNi. This intriguing spin current transport can be explained by the angular momentum transfer mediated by the antiferromagnetic magnons. The results assure that the spin current exerts a torque on the NiO magnetic moments and excites their dynamics. In the talk, recent results will be also discussed.
Spin Seebeck Effect Signals from Antiferromagnets
Prakash, Arati; Brangham, Jack; Yang, Fengyuan; Heremans, Joseph
The Longitudinal Spin Seebeck Effect (LSSE), in which a heat current stimulates spin propagation across an interface between a magnetic material and a normal metal, is well established and observed in ferromagnetic systems. Data have been presented indicating that antiferromagnetic systems could also give rise to LSSE signals. We report here on LSSE signal measured on the Pt/NiO/YIG structure, where NiO is an antiferromagnet. This system is reported to exhibit antiferromagnonic transport. We explore the dependence of the signal on the thickness of the NiO and YIG layers. We also report its temperature dependence, which was not explored before. The results are interpreted in terms of the temperature dependence of the magnon density of states. It appears that magnon modes with energies below about 40 K are most involved in the process, as was the case to the LSSE on YIG itself. Preliminary results using other antiferromagnets and other inverse spin-Hall layers look promising and will also be reported Work supported by ARO- MURI W911NF-14-1-0016.
Model calculation of thermal conductivity in antiferromagnets
Mikhail, I.F.I., E-mail: ifi_mikhail@hotmail.com; Ismail, I.M.M.; Ameen, M.
2015-11-01
A theoretical study is given of thermal conductivity in antiferromagnetic materials. The study has the advantage that the three-phonon interactions as well as the magnon phonon interactions have been represented by model operators that preserve the important properties of the exact collision operators. A new expression for thermal conductivity has been derived that involves the same terms obtained in our previous work in addition to two new terms. These two terms represent the conservation and quasi-conservation of wavevector that occur in the three-phonon Normal and Umklapp processes respectively. They gave appreciable contributions to the thermal conductivity and have led to an excellent quantitative agreement with the experimental measurements of the antiferromagnet FeCl{sub 2}. - Highlights: • The Boltzmann equations of phonons and magnons in antiferromagnets have been studied. • Model operators have been used to represent the magnon–phonon and three-phonon interactions. • The models possess the same important properties as the exact operators. • A new expression for the thermal conductivity has been derived. • The results showed a good quantitative agreement with the experimental data of FeCl{sub 2}.
Optical cryocooling of diamond
Kern, M.; Jeske, J.; Lau, D. W. M.; Greentree, A. D.; Jelezko, F.; Twamley, J.
2017-06-01
The cooling of solids by optical means only using anti-Stokes emission has a long history of research and achievements. Such cooling methods have many advantages ranging from no moving parts or fluids through to operation in vacuum and may have applications to cryosurgery. However, achieving large optical cryocooling powers has been difficult to manage except in certain rare-earth crystals but these are mostly toxic and not biocompatible. Through study of the emission and absorption cross sections we find that diamond, containing either nitrogen vacancy (NV) or silicon vacancy defects, shows potential for optical cryocooling and, in particular, NV doping shows promise for optical refrigeration. We study the optical cooling of doped diamond microcrystals ranging 10-250 μ m in diameter trapped either in vacuum or in water. For the vacuum case we find NV-doped microdiamond optical cooling below room temperature could exceed |Δ T |>10 K for irradiation powers of Pin<100 mW. We predict that such temperature changes should be easily observed via large alterations in the diffusion constant for optically cryocooled microdiamonds trapped in water in an optical tweezer or via spectroscopic signatures such as the zero-phonon line width or Raman line.
Transmission diamond imaging detector
Smedley, John, E-mail: smedley@bnl.gov; Pinelli, Don; Gaoweia, Mengjia [Brookhaven National Laboratory, Upton, NY (United States); Muller, Erik; Ding, Wenxiang; Zhou, Tianyi [Stony Brook University, Stony Brook, NY (United States); Bohon, Jen [Case Center for Synchrotron Biosciences, Center for Proteomics and Bioinformatics, Case Western Reserve University, Cleveland, OH (United States)
2016-07-27
Many modern synchrotron techniques are trending toward use of high flux beams and/or beams which require enhanced stability and precise understanding of beam position and intensity from the front end of the beamline all the way to the sample. For high flux beams, major challenges include heat load management in optics (including the vacuum windows) and a mechanism of real-time volumetric measurement of beam properties such as flux, position, and morphology. For beam stability in these environments, feedback from such measurements directly to control systems for optical elements or to sample positioning stages would be invaluable. To address these challenges, we are developing diamond-based instrumented vacuum windows with integrated volumetric x-ray intensity, beam profile and beam-position monitoring capabilities. A 50 µm thick single crystal diamond has been lithographically patterned to produce 60 µm pixels, creating a >1kilopixel free-standing transmission imaging detector. This device, coupled with a custom, FPGA-based readout, has been used to image both white and monochromatic x-ray beams and capture the last x-ray photons at the National Synchrotron Light Source (NSLS). This technology will form the basis for the instrumented end-station window of the x-ray footprinting beamline (XFP) at NSLS-II.
Presolar Diamond in Meteorites
Amari, Sachiko
2009-01-01
Presolar diamond, the carrier of the isotopically anomalous Xe component Xe-HL, was the first mineral type of presolar dust that was isolated from meteorites. The excesses in the light, p-process only isotopes 124Xe and 126Xe, and in the heavy, r-process only isotopes 134Xe and 136Xe relative to the solar ratios indicate that Xe-HL was produced in supernovae: they are the only stellar source where these two processes are believed to take place. Although these processes occur in supernovae, their physical conditions and timeframes are completely different. Yet the excesses are always correlated in diamond separates from meteorites. Furthermore, the p-process 124Xe/126Xe inferred from Xe-L and the r-process 134Xe/136Xe from Xe-H do not agree with the p-process and r-process ratios derived from the solar system abundance, and the inferred p-process ratio does not agree with those predicted from stellar models. The 'rapid separation scenario', where the separation of Xe and its radiogenic precursors Te and I take...
B. Zhang; X. Lu; Z.X. Qin; H.B. Chang; X.Y. Ruan
2002-01-01
The aims of the work were to study the effect of Ge (0-6wt. %) on the paramagnetic-antiferromagnetic transition and martensitic transformation of Fe-Mn alloy using the susceptibility, microstructure examination, X-ray diffraction (XRD) and lattice parameter measurement. Ge lowers the Neel temperature, TN, and enhances the mag-netic susceptibility X, changing the Pauli paramagnetism above TN to paramagnetism state obeying the Curie Weiss law, which is essentially similar to that of γ-Fe-Mn alloys containing Al or Si; Ge depresses γ → ε martensitic transformation, which attribute to Ge increasing the stacking fault energy; Moreover, Ge increases the lat-tice parameter of 7 phase, and low content Ge increases the lattice parameter of γphase more than that of high Ge content. Comparing Ge(4s2 4p2 ) with Si(3s2 3p2 ) and Al(3s2 3p1), which have the same outer-shell of electron structures, we found that their effects on the martensitic transformation of Fe-Mn alloy are completely different. The result suggests the outer-shell of electron is not the main factor of governing the Ms temperature of Fe-Mn alloy although it is essential in the alloy's antiferromagnetic transition. The relation among the Ms temperature, stacking fault energy and lattice parameter of austenite, has been discussed in brief.
Coalescence-driven magnetic order of the uncompensated antiferromagnetic Co doped ZnO
Ney, V.; Henne, B.; Lumetzberger, J.; Wilhelm, F.; Ollefs, K.; Rogalev, A.; Kovacs, A.; Kieschnick, M.; Ney, A.
2016-12-01
The evolution of the structural and magnetic properties of Co doped ZnO has been investigated over an unprecedented concentration range above the coalescence limit. ZnO films with Co concentrations from 20% to 60% of the cationic lattice have been grown by reactive magnetron sputtering. The wurtzite crystal structure was maintained even for these high dopant concentrations. By measuring the x-ray absorption at the near edge and the linear and circular dichroism of the films at the Zn and Co K edge, it could be shown that Co substitutes predominantly for Zn in the lattice. No indications of metallic Co have been found in the samples. At low Co concentrations, the films are paramagnetic, but with increasing Co content, the films become antiferromagnetically ordered with increasing order temperature. Uncompensated spins, coupled to the antiferromagnetic dopant configurations, lead to a vertical exchange-bias-like effect, which increases with increasing Co concentration. In parallel, the single-ion anisotropy is gradually lost.
Santocanale, Luigi
2002-01-01
A μ-lattice is a lattice with the property that every unary polynomial has both a least and a greatest fix-point. In this paper we define the quasivariety of μ-lattices and, for a given partially ordered set P, we construct a μ-lattice JP whose elements are equivalence classes of games in a preor...
Spinor bose gases in cubic optical lattice
Mobarak, Mohamed Saidan Sayed Mohamed
2014-01-27
In recent years the quantum simulation of condensed-matter physics problems has resulted from exciting experimental progress in the realm of ultracold atoms and molecules in optical lattices. In this thesis we analyze theoretically a spinor Bose gas loaded into a three-dimensional cubic optical lattice. In order to account for different superfluid phases of spin-1 bosons with a linear Zeeman effect, we work out a Ginzburg-Landau theory for the underlying spin-1 Bose-Hubbard model. To this end we add artificial symmetry-breaking currents to the spin-1 Bose-Hubbard Hamiltonian in order to break the global U (1) symmetry. With this we determine a diagrammatic expansion of the grand-canonical free energy up to fourth order in the symmetry-breaking currents and up to the leading non-trivial order in the hopping strength which is of first order. As a cross-check we demonstrate that the resulting grand-canonical free energy allows to recover the mean-field theory. Applying a Legendre transformation to the grand-canonical free energy, where the symmetry-breaking currents are transformed to order parameters, we obtain the effective Ginzburg-Landau action. With this we calculate in detail at zero temperature the Mott insulator-superfluid quantum phase boundary as well as condensate and particle number density in the superfluid phase. We find that both mean-field and Ginzburg-Landau theory yield the same quantum phase transition between the Mott insulator and superfluid phases, but the range of validity of the mean-field theory turns out to be smaller than that of the Ginzburg-Landau theory. Due to this finding we expect that the Ginzburg-Landau theory gives better results for the superfluid phase and, thus, we restrict ourselves to extremize only the effective Ginzburg-Landau action with respect to the order parameters. Without external magnetic field the superfluid phase is a polar (ferromagnetic) state for anti-ferromagnetic (ferromagnetic) interactions, i.e. only the
Tailoring nanocrystalline diamond film properties
Gruen, Dieter M.; McCauley, Thomas G.; Zhou, Dan; Krauss, Alan R.
2003-07-15
A method for controlling the crystallite size and growth rate of plasma-deposited diamond films. A plasma is established at a pressure in excess of about 55 Torr with controlled concentrations of hydrogen up to about 98% by volume, of unsubstituted hydrocarbons up to about 3% by volume and an inert gas of one or more of the noble gases and nitrogen up to about 98% by volume. The volume ratio of inert gas to hydrogen is preferably maintained at greater than about 4, to deposit a diamond film on a suitable substrate. The diamond film is deposited with a predetermined crystallite size and at a predetermined growth rate.
Robust spin transfer torque in antiferromagnetic tunnel junctions
Saidaoui, Hamed Ben Mohamed
2017-04-18
We theoretically study the current-induced spin torque in antiferromagnetic tunnel junctions, composed of two semi-infinite antiferromagnetic layers separated by a tunnel barrier, in both clean and disordered regimes. We find that the torque enabling electrical manipulation of the Néel antiferromagnetic order parameter is out of plane, ∼n×p, while the torque competing with the antiferromagnetic exchange is in plane, ∼n×(p×n). Here, p and n are the Néel order parameter direction of the reference and free layers, respectively. Their bias dependence shows behavior similar to that in ferromagnetic tunnel junctions, the in-plane torque being mostly linear in bias, while the out-of-plane torque is quadratic. Most importantly, we find that the spin transfer torque in antiferromagnetic tunnel junctions is much more robust against disorder than that in antiferromagnetic metallic spin valves due to the tunneling nature of spin transport.
Emergent lattices with geometrical frustration in doped extended Hubbard models
Kaneko, Ryui; Tocchio, Luca F.; Valentí, Roser; Gros, Claudius
2016-11-01
Spontaneous charge ordering occurring in correlated systems may be considered as a possible route to generate effective lattice structures with unconventional couplings. For this purpose we investigate the phase diagram of doped extended Hubbard models on two lattices: (i) the honeycomb lattice with on-site U and nearest-neighbor V Coulomb interactions at 3 /4 filling (n =3 /2 ) and (ii) the triangular lattice with on-site U , nearest-neighbor V , and next-nearest-neighbor V' Coulomb interactions at 3 /8 filling (n =3 /4 ). We consider various approaches including mean-field approximations, perturbation theory, and variational Monte Carlo. For the honeycomb case (i), charge order induces an effective triangular lattice at large values of U /t and V /t , where t is the nearest-neighbor hopping integral. The nearest-neighbor spin exchange interactions on this effective triangular lattice are antiferromagnetic in most of the phase diagram, while they become ferromagnetic when U is much larger than V . At U /t ˜(V/t ) 3 , ferromagnetic and antiferromagnetic exchange interactions nearly cancel out, leading to a system with four-spin ring-exchange interactions. On the other hand, for the triangular case (ii) at large U and finite V', we find no charge order for small V , an effective kagome lattice for intermediate V , and one-dimensional charge order for large V . These results indicate that Coulomb interactions induce [case (i)] or enhance [case(ii)] emergent geometrical frustration of the spin degrees of freedom in the system, by forming charge order.
Ghosh, Pratyay; Verma, Akhilesh Kumar; Kumar, Brijesh
2016-01-01
A spin-1 Heisenberg model on trimerized kagome lattice is studied by doing a low-energy bosonic theory in terms of plaquette triplons defined on its triangular unit cells. The model considered has an intratriangle antiferromagnetic exchange interaction J (set to 1) and two intertriangle couplings J'>0 (nearest neighbor) and J″ (next nearest neighbor; of both signs). The triplon analysis performed on this model investigates the stability of the trimerized singlet ground state (which is exact in the absence of intertriangle couplings) in the J'-J″ plane. It gives a quantum phase diagram that has two gapless antiferromagnetically ordered phases separated by the spin-gapped trimerized singlet phase. The trimerized singlet ground state is found to be stable on J″=0 line (the nearest-neighbor case), and on both sides of it for J″≠0 , in an extended region bounded by the critical lines of transition to the gapless antiferromagnetic phases. The gapless phase in the negative J″ region has a coplanar 120∘ antiferromagnetic order with √{3 }×√{3 } structure. In this phase, all the magnetic moments are of equal length, and the angle between any two of them on a triangle is exactly 120∘. The magnetic lattice in this case has a unit cell consisting of three triangles. The other gapless phase, in the positive J″ region, is found to exhibit a different coplanar antiferromagnetic order with ordering wave vector q =(0 ,0 ) . Here, two magnetic moments in a triangle are of the same magnitude, but shorter than the third. While the angle between two short moments is 120∘-2 δ , it is 120∘+δ between a short and the long one. Only when J″=J' , their magnitudes become equal and the relative angles 120∘. The magnetic lattice in this q =(0 ,0 ) phase has the translational symmetry of the kagome lattice with triangular unit cells of reduced (isosceles) symmetry. This reduction in the point-group symmetry is found to show up as a difference in the intensities of
Ground state configurations in antiferromagnetic ultrathin films with dipolar anisotropy
Leon, H., E-mail: hleon@imre.oc.uh.cu [Instituto de Ciencia y Tecnologia de Materiales, Universidad de La Habana, Zapata e/ Mazon y G. Vedado, 10400 La Habana (Cuba)
2013-02-15
The formalism developed in a previous work to calculate the dipolar energy in quasi-two-dimensional crystals with ferromagnetic order is now extended to collinear antiferromagnetic order. Numerical calculations of the dipolar energy are carried out for systems with tetragonally distorted fcc [001] structures, the case of NiO and MnO ultrathin film grown in non-magnetic substrates, where the magnetic phase is a consequence of superexchange and dipolar interactions. The employed approximation allows to demonstrate that dipolar coupling between atomic layers is responsible for the orientation of the magnetization when it differs from the one in a single layer. The ground state energy of a given NiO or MnO film is found to depend not only on the strain, but also on how much the interlayer separation and the 2D lattice constant are changed with respect to the ideal values corresponding to the non-distorted cubic structure. Nevertheless, it is shown that the orientation of the magnetization in the magnetic phase of any of these films is determined by the strain exclusively. A striped phase with the magnetization along the [112{sup Macron }] direction appears as the ground state configuration of NiO and MnO ultrathin films. In films with equally oriented stripes along the layers this magnetic phase is twofold degenerate, while in films with multidomain layers it is eightfold degenerate. These results are not in contradiction with experimentally observed out-of-plane or in-plane magnetization of striped phases in NiO and MnO ultrathin films. - Highlights: Black-Right-Pointing-Pointer Dipolar energy in collinear antiferromagnetic ultrathin films is calculated. Black-Right-Pointing-Pointer Numerical results are presented for distorted fcc [001] structures. Black-Right-Pointing-Pointer The lowest energy of a system depends on how the tetragonal distortion is achieved. Black-Right-Pointing-Pointer A striped phase with magnetization in the [112{sup Macron }] direction is the
Spin-S kagome quantum antiferromagnets in a field with tensor networks
Picot, Thibaut; Ziegler, Marc; Orús, Román; Poilblanc, Didier
2016-02-01
Spin-S Heisenberg quantum antiferromagnets on the kagome lattice offer, when placed in a magnetic field, a fantastic playground to observe exotic phases of matter with (magnetic analogs of) superfluid, charge, bond, or nematic orders, or a coexistence of several of the latter. In this context, we have obtained the (zero-temperature) phase diagrams up to S =2 directly in the thermodynamic limit owing to infinite projected entangled pair states, a tensor network numerical tool. We find incompressible phases characterized by a magnetization plateau versus field and stabilized by spontaneous breaking of point group or lattice translation symmetry(ies). The nature of such phases may be semiclassical, as the plateaus at the 1/3th ,(1-2/9S)th, and (1-1/9S)th of the saturated magnetization (the latter followed by a macroscopic magnetization jump), or fully quantum as the spin-1/2 1/9 plateau exhibiting a coexistence of charge and bond orders. Upon restoration of the spin rotation U (1 ) symmetry, a finite compressibility appears, although lattice symmetry breaking persists. For integer spin values we also identify spin gapped phases at low enough fields, such as the S =2 (topologically trivial) spin liquid with no symmetry breaking, neither spin nor lattice.
Fabrication and Mechanical Characterisation of Titanium Lattices with Graded Porosity
William van Grunsven
2014-08-01
Full Text Available Electron Beam Melting (EBM is an Additive Manufacturing technique which can be used to fabricate complex structures from alloys such as Ti6Al4V, for example for orthopaedic applications. Here we describe the use of EBM for the fabrication of a novel Ti6Al4V structure of a regular diamond lattice incorporating graded porosity, achieved via changes in the strut cross section thickness. Scanning Electron Microscopy and micro computed tomography analysis confirmed that generally EBM reproduced the CAD design of the lattice well, although at smaller strut sizes the fabricated lattice produced thicker struts than the model. Mechanical characterisation of the lattice in uniaxial compression showed that its behaviour under compression along the direction of gradation can be predicted to good accuracy with a simple rule of mixtures approach, knowing the properties and the behaviour of its constituent layers.
B K Sahoo; B N Panda
2011-10-01
The effect of hybridization of conduction electrons and f-level on superconductivity (SC) and antiferromagnetism (AFM) in the coexistent phase of rare-earth nickel borocarbide superconductors (Ni2B2C) is reported. The Hamiltonian of the system is a mean ﬁeld one and has been solved by writing equations of motion for the single-particle Green functions. It is assumed that superconductivity arises due to BCS pairing mechanism in the presence of antiferromagnetism in nickel lattices of Ni2B2 plane. The expressions for superconducting and antiferromagnetic order parameters are derived using double time electron Green functions. The quasiparticle energy bands are plotted and the nature of band dispersion of the quasiparticles is studied.
Akamatsu, Hirofumi; Kumagai, Yu; Oba, Fumiyasu; Fujita, Koji; Murakami, Hideo; Tanaka, Katsuhisa; Tanaka, Isao
2011-06-01
A superexchange mechanism between Eu2+ 4f spins via the 3d states of nonmagnetic Ti4+ ions is proposed through first-principles calculations based on a hybrid Hartree-Fock density functional approach to explain G-type antiferromagnetism in EuTiO3. This mechanism is supported by systematic calculations for related Eu2+-based perovskite oxides. In EuTiO3, the competition between the antiferromagnetic superexchange and an indirect ferromagnetic exchange via the Eu 5d states leads to a delicate balance between antiferromagnetic and ferromagnetic phases. The superexchange mechanism involving the Ti 3d states hints at the microscopic origin of the strong spin-lattice coupling in EuTiO3.
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2008-01-01
对于酒的品味不仅仅在酒本身所散发出的醉人魅力，自古以来，拥有艺术品般精湛做工、华美造犁的盛酒器皿也和酒一样流传千古。The Diamond Standard Vodka以“奢侈”、“豪华”作为卖点，除了散发着北欧风格的高贵气质外，由原产自奥地利的施华洛廿奇水晶制成25mm的瓶身更让它身价倍增。以钻石命名的它使用了钻石过滤专利系统，
Dynamic magnetic hysteresis and nonlinear susceptibility of antiferromagnetic nanoparticles
Kalmykov, Yuri P.; Ouari, Bachir; Titov, Serguey V.
2016-08-01
The nonlinear ac stationary response of antiferromagnetic nanoparticles subjected to both external ac and dc fields of arbitrary strength and orientation is investigated using Brown's continuous diffusion model. The nonlinear complex susceptibility and dynamic magnetic hysteresis (DMH) loops of an individual antiferromagnetic nanoparticle are evaluated and compared with the linear regime for extensive ranges of the anisotropy, the ac and dc magnetic fields, damping, and the specific antiferromagnetic parameter. It is shown that the shape and area of the DMH loops of antiferromagnetic particles are substantially altered by applying a dc field that permits tuning of the specific magnetic power loss in the nanoparticles.
Dynamics of antiferromagnetic skyrmion driven by the spin Hall effect
Jin, Chendong; Song, Chengkun; Wang, Jianbo; Liu, Qingfang
2016-10-01
Magnetic skyrmion moved by the spin-Hall effect is promising for the application of the generation racetrack memories. However, the Magnus force causes a deflected motion of skyrmion, which limits its application. Here, we create an antiferromagnetic skyrmion by injecting a spin-polarized pulse in the nanostripe and investigate the spin Hall effect-induced motion of antiferromagnetic skyrmion by micromagnetic simulations. In contrast to ferromagnetic skyrmion, we find that the antiferromagnetic skyrmion has three evident advantages: (i) the minimum driving current density of antiferromagnetic skyrmion is about two orders smaller than the ferromagnetic skyrmion; (ii) the velocity of the antiferromagnetic skyrmion is about 57 times larger than the ferromagnetic skyrmion driven by the same value of current density; (iii) antiferromagnetic skyrmion can be driven by the spin Hall effect without the influence of Magnus force. In addition, antiferromagnetic skyrmion can move around the pinning sites due to its property of topological protection. Our results present the understanding of antiferromagnetic skyrmion motion driven by the spin Hall effect and may also contribute to the development of antiferromagnetic skyrmion-based racetrack memories.
V.V. Kulish
2015-06-01
Full Text Available The paper investigates the antiferromagnetic vector distribution in an antiferromagnetic film with a system of antidots. A static distribution of the antiferromagnetic vector is written and a method – based on the minimization of the antiferromagnet energy – that allows reducing the number of boundary conditions required for finding the constants of this distribution is proposed. Equations for the distribution constants are obtained for the both cases of minimizing the antiferromagnet energy by one and by two distribution constants that enter the expression for the antiferromagnet energy. The method is illustrated on a system of one isolated antidot. For such system, one additional condition – for the case when two boundary conditions on the surface of the antidot are given – and two additional conditions – for the case when one boundary condition on the surface of the antidot is given – on the distribution constants are written.
Generation of Nitrogen-Vacancy Centers in Diamond with Ion Implantation
CUI Jin-Ming; CHEN Xiang-Dong; FAN Le-Le; GONG Zhao-Jun; ZOU Chong-Wen; SUN Fang-Wen; HAN Zheng-Fu; GUO Guang-Can
2012-01-01
Nitrogen-vacancy defect color centers are created in a high purity single crystal diamond by nitrogen-ion implantation.Both optical spectrum and optically detected magnetic resonance are measured for these artificial quantum emitters.Moreover,with a suitable mask,a lattice composed of nitrogen-vacancy centers is fabricated.Rabi oscillation driven by micro-waves is carried out to show the quality of the ion implantation and potential in quantum manipulation.Along with compatible standard lithography,such an implantation technique shows high potential in future to make structures with nitrogen-vacancy centers for diamond photonics and integrated photonic quantum chip.
Pulse laser induced graphite-to-diamond phase transition: the role of quantum electronic stress
Wang, ZhengFei; Liu, Feng
2017-02-01
First-principles calculations show that the pulse laser induced graphite-to-diamond phase transition is related to the lattice stress generated by the excited carriers, termed as "quantum electronic stress (QES)". We found that the excited carriers in graphite generate a large anisotropic QES that increases linearly with the increasing carrier density. Using the QES as a guiding parameter, structural relaxation spontaneously transforms the graphite phase into the diamond phase, as the QES is reduced and minimized. Our results suggest that the concept of QES can be generally applied as a good measure to characterize the pulse laser induced phase transitions, in analogy to pressure induced phase transitions.
Study of double triple bend achromat (DTBA) lattice for a 3GeV light source
Alekou, Androula; Carmignani, Nicola; Liuzzo, Simone Maria; Raimondi, Pantaleo; Pulampong, Thapakron; Walker, Richard
2017-01-01
Starting from the concepts of the Hybrid Multi Bend Achromat (HMBA) lattice developed at ESRF and of the Double-Double Bend Achromat(DDBA) lattice developed at Diamond, we present a new cell tha tincludes all the advantages of the two designs. The resulting Double Triple Bend Achromat(DTBA) cel lallows for a natural horizontal emittance of less than 100pm with a large dynamic aperture and lifetime. It includes two straight sections, for insertion devices, ﬁve and three meters long. The lattice is consistent with the engineering design developed for the ESRF-EBS lattice and the layout and user requirements of Diamond. The characteristics of the cell are presented together with the results of the optimisation process.
Helium and carbon isotopes in Indian diamonds
Wiens, R.; Lal, D.; Craig, H.
1990-09-01
Helium and carbon isotope measurements in Indian diamonds (from Andhra Pradesh) were carried out using samples that included mined diamonds from primary kimberlite source rocks and alluvial diamonds from river gravel. The He and C isotope concentrations in diamonds from these two sources were compared, and the Indian diamonds were compared to those from other regions. Results indicate that most of the He-3 in the alluvial diamonds is of cosmogenic origin and that the alluvial diamonds may also have a significant He-4 component due to alpha particles implanted during storage in a secondary matrix. One diamond, a mined kimberlite specimen, was found to have the lowest He-4 content (0.018 microcc/g) so far recorded in diamonds.
Dynamic scaling of the restoration of rotational symmetry in Heisenberg quantum antiferromagnets
Weinberg, Phillip; Sandvik, Anders W.
2017-08-01
We apply imaginary-time evolution with the operator e-τ H to study relaxation dynamics of gapless quantum antiferromagnets described by the spin-rotation-invariant Heisenberg Hamiltonian H . Using quantum Monte Carlo simulations to obtain unbiased results, we propagate an initial state with maximal order parameter msz (the staggered magnetization) in the z spin direction and monitor the expectation value 〈ms〉 as a function of imaginary time τ . Results for different system sizes (lengths) L exhibit an initial essentially size independent relaxation of 〈ms〉 toward its value in the infinite-size spontaneously symmetry broken state, followed by a strongly size dependent final decay to zero when the O (3 ) rotational symmetry of the order parameter is restored. We develop a generic finite-size scaling theory that shows the relaxation time diverges asymptotically as Lz, where z is the dynamic exponent of the low-energy excitations. We use the scaling theory to develop a practical way of extracting the dynamic exponent from the numerical finite-size data, systematically eliminating scaling corrections. We apply the method to spin-1 /2 Heisenberg antiferromagnets on two different lattice geometries: the standard two-dimensional (2D) square lattice and a site-diluted 2D square lattice at the percolation threshold. In the 2D case we obtain z =2.001 (5 ) , which is consistent with the known value z =2 , while for the site-diluted lattice we find z =3.90 (1 ) or z =2.056 (8 ) Df , where Df=91 /48 is the fractal dimensionality of the percolating system. This is an improvement on previous estimates of z ≈3.7 . The scaling results also show a fundamental difference between the two cases; for the 2D square lattice, the data can be collapsed onto a common scaling function even when 〈ms〉 is relatively large, reflecting the Anderson tower of quantum rotor states with a common dynamic exponent z =2 . For the diluted 2D square lattice, the scaling works well only for
Signal and noise of Diamond Pixel Detectors at High Radiation Fluences
Tsung, Jieh-Wen; Hügging, Fabian; Kagan, Harris; Krüger, Hans; Wermes, Norbert
2012-01-01
CVD diamond is an attractive material option for LHC vertex detectors because of its strong radiation-hardness causal to its large band gap and strong lattice. In particular, pixel detectors operating close to the interaction point profit from tiny leakage currents and small pixel capacitances of diamond resulting in low noise figures when compared to silicon. On the other hand, the charge signal from traversing high energy particles is smaller in diamond than in silicon by a factor of about 2.2. Therefore, a quantitative determination of the signal-to-noise ratio (S/N) of diamond in comparison with silicon at fluences in excess of 10$^{15}$ n$_{eq}$ cm$^{-2}$, which are expected for the LHC upgrade, is important. Based on measurements of irradiated diamond sensors and the FE-I4 pixel readout chip design, we determine the signal and the noise of diamond pixel detectors irradiated with high particle fluences. To characterize the effect of the radiation damage on the materials and the signal decrease, the chang...
Quantum photonic networks in diamond
Lončar, Marko
2013-02-01
Advances in nanotechnology have enabled the opportunity to fabricate nanoscale optical devices and chip-scale systems in diamond that can generate, manipulate, and store optical signals at the single-photon level. In particular, nanophotonics has emerged as a powerful interface between optical elements such as optical fibers and lenses, and solid-state quantum objects such as luminescent color centers in diamond that can be used effectively to manipulate quantum information. While quantum science and technology has been the main driving force behind recent interest in diamond nanophotonics, such a platform would have many applications that go well beyond the quantum realm. For example, diamond\\'s transparency over a wide wavelength range, large third-order nonlinearity, and excellent thermal properties are of great interest for the implementation of frequency combs and integrated Raman lasers. Diamond is also an inert material that makes it well suited for biological applications and for devices that must operate in harsh environments. Copyright © Materials Research Society 2013.
Switching of antiferromagnetic chains with magnetic pulses
Tao, Kun; Polyakov, Oleg P.; Stepanyuk, Valeri S.
2016-04-01
Recent experimental studies have demonstrated the possibility of information storage in short antiferromagnetic chains on an insulator substrate [S. Loth et al., Science 335, 196 (2012), 10.1126/science.1214131]. Here, using the density functional theory and atomistic spin dynamics simulations, we show that a local magnetic control of such chains with a magnetic tip and magnetic pulses can be used for fast switching of their magnetization. Furthermore, by changing the position of the tip one can engineer the magnetization dynamics of the chains.
High-Tc spin superfluidity in antiferromagnets.
Bunkov, Yu M; Alakshin, E M; Gazizulin, R R; Klochkov, A V; Kuzmin, V V; L'vov, V S; Tagirov, M S
2012-04-27
We report the observation of the unusual behavior of induction decay signals in antiferromagnetic monocrystals with Suhl-Nakamura interactions. The signals show the formation of the Bose-Einstein condensation (BEC) of magnons and the existence of spin supercurrent, in complete analogy with the spin superfluidity in the superfluid (3)He and the atomic BEC of quantum gases. In the experiments described here, the temperature of the magnon BEC is a thousand times larger than in the superfluid (3)He. It opens a possibility to apply the spin supercurrent for various magnetic spintronics applications.
Spin liquid nature in the Heisenberg J1-J2 triangular antiferromagnet
Iqbal, Yasir; Hu, Wen-Jun; Thomale, Ronny; Poilblanc, Didier; Becca, Federico
2016-04-01
We investigate the spin-1/2 Heisenberg model on the triangular lattice in the presence of nearest-neighbor J1 and next-nearest-neighbor J2 antiferromagnetic couplings. Motivated by recent findings from density-matrix renormalization group (DMRG) claiming the existence of a gapped spin liquid with signatures of spontaneously broken lattice point group symmetry [Zhu and White, Phys. Rev. B 92, 041105 (2015), 10.1103/PhysRevB.92.041105 and Hu, Gong, Zhu, and Sheng, Phys. Rev. B 92, 140403 (2015), 10.1103/PhysRevB.92.140403], we employ the variational Monte Carlo (VMC) approach to analyze the model from an alternative perspective that considers both magnetically ordered and paramagnetic trial states. We find a quantum paramagnet in the regime 0.08 ≲J2/J1≲0.16 , framed by 120∘ coplanar (stripe collinear) antiferromagnetic order for smaller (larger) J2/J1 . By considering the optimization of spin-liquid wave functions of a different gauge group and lattice point group content as derived from Abrikosov mean-field theory, we obtain the gapless U(1 ) Dirac spin liquid as the energetically most preferable state in comparison to all symmetric or nematic gapped Z2 spin liquids so far advocated by DMRG. Moreover, by the application of few Lanczos iterations, we find the energy to be the same as the DMRG result within error bars. To further resolve the intriguing disagreement between VMC and DMRG, we complement our methodological approach by the pseudofermion functional renormalization group (PFFRG) to compare the spin structure factors for the paramagnetic regime calculated by VMC, DMRG, and PFFRG. This model promises to be an ideal test bed for future numerical refinements in tracking the long-range correlations in frustrated magnets.
Measuring spin correlations in optical lattices using superlattice potentials
Pedersen, Kim Georg Lind; Andersen, Brian Møller; Bruun, Georg Morten;
2011-01-01
We suggest two experimental methods for probing both short- and long-range spin correlations of atoms in optical lattices using superlattice potentials. The first method involves an adiabatic doubling of the periodicity of the underlying lattice to probe neighboring singlet (triplet) correlations...... for fermions (bosons) by the occupation of the resulting vibrational ground state. The second method utilizes a time-dependent superlattice potential to generate spin-dependent transport by any number of prescribed lattice sites, and probes correlations by the resulting number of doubly occupied sites....... For experimentally relevant parameters, we demonstrate how both methods yield large signatures of antiferromagnetic correlations of strongly repulsive fermionic atoms in a single shot of the experiment. Lastly, we show how this method may also be applied to probe d-wave pairing, a possible ground-state candidate...
Hydrogenated Black Diamond: An Electrical Study
Williams, O.A.; Jackman, R.B. [Electronic and Electrical Engineering, University College London, Torrington Place, London, WC1E 7JE (United Kingdom); Nebel, C.E. [Walter Schottky Institut, Technische Universitaet Muenchen, Am Coulombwall, 85748 Garching (Germany)
2002-10-16
Hydrogen surface conductivity has been a controversial subject since its discovery. Initial plasma treatments on single crystal diamond and polycrystalline diamond have lead to the widespread use of this material in active electronics. However, ''Black'' polycrystalline diamond, usually termed ''Thermal Management Grade'', shows carrier concentration and mobility values similar to both white polycrystalline diamond and single crystal material. Schottky contacts have also been fabricated and show promising characteristics. Black diamond can be grown considerably faster than white diamond and is hence much cheaper. (Abstract Copyright [2002], Wiley Periodicals, Inc.)
Tajiri, Takeyoshi; Takahashi, Shun; Tandaechanurat, Aniwat; Iwamoto, Satoshi; Arakawa, Yasuhiko
2014-01-01
We design a three-dimensional (3D) photonic crystal (PC) nanocavity based on a \\langle 110\\rangle -layered diamond structure. The designed structure, comprised of self-sustainable layers, is suitable for fabrication by layer stacking techniques. Quality factors (Q-factors) of nanocavities were calculated for the \\langle 110\\rangle -layered diamond and a commonly-used woodpile structures, both of which are generated from the same diamond lattice with a lattice constant adiamond. The Q-factor of the designed nanocavity can reach as high as 230,000 with 35 stacked layers and a square in-plane PC area of the length of one side of 5\\sqrt{2} a^{\\text{diamond}}. This is 1.5 times higher than that of a 3D PC nanocavity based on the woodpile structure with the same in-plane PC size and with the same number of stacked layers. The higher Q-factor in the \\langle 110\\rangle -layered diamond structure originates from its stronger in-plane light confinement over the woodpile structure. The \\langle 110\\rangle -layered diamond structure will be beneficial for improving experimentally attainable Q-factors of 3D PC nanocavities particularly fabricated by a micromanipulation method.
Diamonds: Exploration, mines and marketing
Read, George H.; Janse, A. J. A. (Bram)
2009-11-01
The beauty, value and mystique of exceptional quality diamonds such as the 603 carat Lesotho Promise, recovered from the Letseng Mine in 2006, help to drive a multi-billion dollar diamond exploration, mining and marketing industry that operates in some 45 countries across the globe. Five countries, Botswana, Russia, Canada, South Africa and Angola account for 83% by value and 65% by weight of annual diamond production, which is mainly produced by four major companies, De Beers, Alrosa, Rio Tinto and BHP Billiton (BHPB), which together account for 78% by value and 72% by weight of annual diamond production for 2007. During the last twelve years 16 new diamond mines commenced production and 4 re-opened. In addition, 11 projects are in advanced evaluation and may begin operations within the next five years. Exploration for diamondiferous kimberlites was still energetic up to the last quarter of 2008 with most work carried out in Canada, Angola, Democratic Republic of the Congo (DRC) and Botswana. Many kimberlites were discovered but no new economic deposits were outlined as a result of this work, except for the discovery and possible development of the Bunder project by Rio Tinto in India. Exploration methods have benefitted greatly from improved techniques of high resolution geophysical aerial surveying, new research into the geochemistry of indicator minerals and further insights into the formation of diamonds and the relation to tectonic/structural events in the crust and mantle. Recent trends in diamond marketing indicate that prices for rough diamonds and polished goods were still rising up to the last quarter of 2008 and subsequently abruptly sank in line with the worldwide financial crisis. Most analysts predict that prices will rise again in the long term as the gap between supply and demand will widen because no new economic diamond discoveries have been made recently. The disparity between high rough and polished prices and low share prices of publicly
Genetic Types of Diamond Mineralization
A.A.MARAKUSHEV; 桑隆康; 等
1998-01-01
The paper describes the proposed models of diamond formation both in meteorites and in kimberlite and lamproite bodies.metamorphic complexes and explosive-ring structures ("astroblemes"),The diamond distribution in meteorites(chondrites,iron meteorites and ureilites)is restricted to taente-kamasite phase.The diamond generation here is tied up with the first stage of evolution of the planets,This stage is characterized by high pressure of hydrogen. leading to the formation of the planet envelope,The second stage of planet evolution began with the progressive imopoverishment of their atmospheres in hydrogen due to its predominant emission into the space and to progressive development of oxidative conditions.The model appears to have proved the relict nature of diamond mineraolization in meteorites.Diamond and other high-pressure minerals(its"satellites") were crystallized without any exception in the early intratelluric stages of peridotite and eclogite-pyroxenite magma evolution just before the magma intrusion into the higher levels of the mantle and crust where diamond is not thermodynamically stable,The ultramafic intrusive bodies(bearing rich relict diamonds)in the dase of a platform paaear to be the substrata for the formation of kimberlite-lamproite magma chambers as a result of magmatic replacement.The model explains the polyfacial nature of diamondiferous eclotgites,pyroxenites and peridotites and discusses the process of inheritance of their diamond mineralization by kimberlites and lamproites.Dimond oproductivity of metamorthic complexes is originated by the inheritance of their diamonds from the above-mentioned primary diamondiferous rocks.Large diamondiferous explosive-ring structures were formed by high-energy endogenic explosion of fluid which came from the Earth's core.This high energy differs endogenic impactogenesis from explosive volcanism.It proceeds at very high temperature to create diaplectic galsses(monomineral pseudomorphs)-the product of
Parente, Walter E.F.; Pacobahyba, J.T.M.; Araújo, Ijanílio G. [Departamento de Física, Universidade Federal de Roraima, BR 174, Km 12. Bairro Monte Cristo. CEP: 69300-000 Boa Vista, Roraima (Brazil); Neto, Minos A., E-mail: minos@pq.cnpq.br [Universidade Federal do Amazonas, Departamento de Física, 3000, Japiim, 69077-000, Manaus-AM (Brazil); Ricardo de Sousa, J. [Universidade Federal do Amazonas, Departamento de Física, 3000, Japiim, 69077-000, Manaus-AM (Brazil); National Institute of Science and Technology for Complex Systems, 3000, Japiim, 69077-000, Manaus-AM (Brazil); Akinci, Ümit [Department of Physics, Dokuz Eylül University, Tr-35160 Izmir (Turkey)
2014-04-15
In this paper we study the quantum spin-1/2 anisotropic Heisenberg antiferromagnet model in the presence of a Dzyaloshinskii–Moriya interaction (D) and a uniform longitudinal (H) magnetic field. Using the effective-field theory with a finite cluster N=2 spin (EFT-2) we calculate the phase diagrams in the H−T and D−T planes on a simple cubic lattice (z=6). We have only observed second order phase transitions for values between Δ∈[0,1], where the cases were analysed: Ising (Δ=1), anisotropic Heisenberg (Δ=0.6) and isotropic Heisenberg (Δ=0). - Highlights: • Anisotropic Heisenberg antiferromagnet on a simple cubic lattice. • Effective-field theory. • Dzyaloshinskii–Moriya interaction.
Study of magnetic properties of spin-dependent Falicov-Kimball model on a triangular lattice
Kumar, Sant; Yadav, Umesh K.; Maitra, Tulika; Singh, Ishwar
2013-02-01
Numerical diagonalization technique and Monte-Carlo simulation algorithm is used to study the ground state properties of spin-dependent Falicov-Kimball model (FKM) on a triangular lattice for 1/3 filling of itinerant (d) and localized (f) electrons. We have found that the ground state configurations are of long range Neel ordered antiferromagnetic, ferromagnetic or mixture of anti-ferromagnetic and ferromagnetic type for different values of exchange correlation (J). The magnetization of d and f-electrons increases with increasing the exchange correlation (J) between d and f-electrons and then decreases with further increasing the value of J.
Antiferromagnetic phase diagram of the cuprate superconductors
Nunes, L. H. C. M.; Teixeira, A. W.; Marino, E. C.
2017-02-01
Taking the spin-fermion model as the starting point for describing the cuprate superconductors, we obtain an effective nonlinear sigma-field hamiltonian, which takes into account the effect of doping in the system. We obtain an expression for the spin-wave velocity as a function of the chemical potential. For appropriate values of the parameters we determine the antiferromagnetic phase diagram for the YBa2Cu3O6+x compound as a function of the dopant concentration in good agreement with the experimental data. Furthermore, our approach provides a unified description for the phase diagrams of the hole-doped and the electron doped compounds, which is consistent with the remarkable similarity between the phase diagrams of these compounds, since we have obtained the suppression of the antiferromagnetic phase as the modulus of the chemical potential increases. The aforementioned result then follows by considering positive values of the chemical potential related to the addition of holes to the system, while negative values correspond to the addition of electrons.
Campos, R G; Campos, Rafael G.; Tututi, Eduardo S.
2002-01-01
It is shown that the nonlocal Dirac operator yielded by a lattice model that preserves chiral symmetry and uniqueness of fields, approaches to an ultralocal and invariant under translations operator when the size of the lattice tends to zero.
New integrable lattice hierarchies
Pickering, Andrew [Area de Matematica Aplicada, ESCET, Universidad Rey Juan Carlos, c/ Tulipan s/n, 28933 Mostoles, Madrid (Spain); Zhu Zuonong [Departamento de Matematicas, Universidad de Salamanca, Plaza de la Merced 1, 37008 Salamanca (Spain) and Department of Mathematics, Shanghai Jiao Tong University, Shanghai 200030 (China)]. E-mail: znzhu2@yahoo.com.cn
2006-01-23
In this Letter we give a new integrable four-field lattice hierarchy, associated to a new discrete spectral problem. We obtain our hierarchy as the compatibility condition of this spectral problem and an associated equation, constructed herein, for the time-evolution of eigenfunctions. We consider reductions of our hierarchy, which also of course admit discrete zero curvature representations, in detail. We find that our hierarchy includes many well-known integrable hierarchies as special cases, including the Toda lattice hierarchy, the modified Toda lattice hierarchy, the relativistic Toda lattice hierarchy, and the Volterra lattice hierarchy. We also obtain here a new integrable two-field lattice hierarchy, to which we give the name of Suris lattice hierarchy, since the first equation of this hierarchy has previously been given by Suris. The Hamiltonian structure of the Suris lattice hierarchy is obtained by means of a trace identity formula.
Charge Stripes and Antiferromagnetism in Copper-Oxide Superconductors
Tranquada, J.M.
1997-12-31
Superconducting cuprate compounds are obtained by doping holes into antiferromagnetic insulators. Neutron scattering studies have provided evidence that the doped holes tend to segregate into charge stripes, which act like domain walls between antiferromagnetic regions. The interaction between the spatially segregated holes and the magnetic domains may be responsible for the strong pairing interaction found in the cuprates.
Nematic antiferromagnetic states in bulk FeSe
Liu, Kai; Lu, Zhong-Yi; Xiang, Tao
2016-05-01
The existence of nematic order, which breaks the lattice rotational symmetry with nonequivalent a and b axes in iron-based superconductors, is a well-established experimental fact. An antiferromagnetic (AFM) transition is accompanying this order, observed in nearly all parent compounds, except bulk FeSe. The absence of the AFM order in FeSe casts doubt on the magnetic mechanism of iron-based superconductivity, since the nematic order is believed to be driven by the same interaction that is responsible for the superconducting pairing in these materials. Here we show, through systematic first-principles electronic structure calculations, that the ground state of FeSe is in fact strongly AFM correlated but without developing a magnetic long-range order. Actually, there are a series of staggered n -mer AFM states with corresponding energies below that of the single stripe AFM state, which is the ground state for the parent compounds of most iron-based superconductors. Here, the staggered n -mer (n any integer >1 ) means a set of n adjacent parallel spins on a line along the b axis with antiparallel spins between n -mers along both a and b axes. Moreover, different n -mers can antiparallelly mix with each other to coexist. Among all the states, we find that the lowest energy states formed by the staggered dimer, staggered trimer, and their random antiparallel aligned spin states along the b axis are quasidegenerate. The thermal average of these states does not show any magnetic long-range order, but it does possess a hidden one-dimensional AFM order along the a axis, which can be detected by elastic neutron scattering measurements. Our finding gives a natural account for the absence of long-range magnetic order and suggests that the nematicity is driven predominantly by spin fluctuations even in bulk FeSe, providing a unified description on the phase diagram of iron-based superconductors.
Sober Topological Molecular Lattices
张德学; 李永明
2003-01-01
A topological molecular lattice (TML) is a pair (L, T), where L is a completely distributive lattice and r is a subframe of L. There is an obvious forgetful functor from the category TML of TML's to the category Loc of locales. In this note,it is showed that this forgetful functor has a right adjoint. Then, by this adjunction,a special kind of topological molecular lattices called sober topological molecular lattices is introduced and investigated.
Classical Spin Liquid on the Maximally Frustrated Honeycomb Lattice
Rehn, J.; Sen, Arnab; Damle, Kedar; Moessner, R.
2016-10-01
We show that the honeycomb Heisenberg antiferromagnet with J1/2 =J2=J3, where J1 , J2 , and J3 are first-, second-, and third-neighbor couplings, respectively, forms a classical spin liquid with pinch-point singularities in the structure factor at the Brillouin zone corners. Upon dilution with nonmagnetic ions, fractionalized degrees of freedom carrying 1 /3 of the free moment emerge. Their effective description in the limit of low temperature is that of spins randomly located on a triangular lattice, with a frustrated sublattice-sensitive interaction of long-ranged logarithmic form. The X Y version of this magnet exhibits nematic thermal order by disorder. This comes with a clear experimental diagnostic in neutron scattering, which turns out to apply also to the case of the celebrated planar order by disorder of the kagome Heisenberg antiferromagnet.
Bilinear-biquadratic anisotropic Heisenberg model on a triangular lattice
Pires, A.S.T., E-mail: antpires@fisica.ufmg.br
2013-08-15
Motivated by the fact that the study of disordered phases at zero temperature is of great interest, I study the spin-one quantum antiferromagnet with a next-nearest neighbor interaction on a triangular lattice with bilinear and biquadratic exchange interactions and a single ion anisotropy, using a SU(3) Schwinger boson mean-field theory. I calculate the critical properties, at zero temperature, for values of the single ion anisotropy parameter D above a critical value D{sub C}, where a quantum phase transition takes place from a higher D disordered phase to a lower D ordered phase. - Highlights: • The quantum phase transition of the bilinear-biquadratic anisotropic antiferromagnet is studied. • The effect of competing interaction is analyzed. • The zero temperature phase diagram is obtained.
The evaluation of radiation damage parameter for CVD diamond
Grilj, V.; Skukan, N.; Jakšić, M.; Pomorski, M.; Kada, W.; Kamiya, T.; Ohshima, T.
2016-04-01
There are a few different phenomenological approaches that aim to track the dependence of signal height in irradiated solid state detectors on the fluence of damaging particles. However, none of them are capable to provide a unique radiation hardness parameter that would reflect solely the material capability to withstand high radiation environment. To extract such a parameter for chemical vapor deposited (CVD) diamond, two different diamond detectors were irradiated with proton beams in MeV energy range and subjected afterwards to ion beam induced charge (IBIC) analysis. The change in charge collection efficiency (CCE) due to defects produced was investigated in context of a theoretical model that was developed on the basis of the adjoint method for linearization of the continuity equations of electrons and holes. Detailed modeling of measured data resulted with the first known value of the kσ product for diamond, where k represents the number of charge carriers' traps created per one simulated primary lattice vacancy and σ represents the charge carriers' capture cross section. As discussed in the text, this product could be considered as a true radiation damage parameter.
Thermal diffusion boron doping of single-crystal natural diamond
Seo, Jung-Hun; Wu, Henry; Mikael, Solomon; Mi, Hongyi; Blanchard, James P.; Venkataramanan, Giri; Zhou, Weidong; Gong, Shaoqin; Morgan, Dane; Ma, Zhenqiang
2016-05-01
With the best overall electronic and thermal properties, single crystal diamond (SCD) is the extreme wide bandgap material that is expected to revolutionize power electronics and radio-frequency electronics in the future. However, turning SCD into useful semiconductors requires overcoming doping challenges, as conventional substitutional doping techniques, such as thermal diffusion and ion implantation, are not easily applicable to SCD. Here we report a simple and easily accessible doping strategy demonstrating that electrically activated, substitutional doping in SCD without inducing graphitization transition or lattice damage can be readily realized with thermal diffusion at relatively low temperatures by using heavily doped Si nanomembranes as a unique dopant carrying medium. Atomistic simulations elucidate a vacancy exchange boron doping mechanism that occurs at the bonded interface between Si and diamond. We further demonstrate selectively doped high voltage diodes and half-wave rectifier circuits using such doped SCD. Our new doping strategy has established a reachable path toward using SCDs for future high voltage power conversion systems and for other novel diamond based electronic devices. The novel doping mechanism may find its critical use in other wide bandgap semiconductors.
Thermal characterization and properties of a copper-diamond composite
Yang, Pin [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Chavez, Thomas P. [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); DiAntonio, Christopher Brian [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Coker, Eric Nicholas [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
2014-09-01
The thermal properties of a commercial copper-diamond composite were measured from below -50°C to above 200°C. The results of thermal expansion, heat capacity, and thermal diffusivity were reported. These data were used to calculate the thermal conductivity of the composite as a function of temperature in the thickness direction. These results are compared with estimated values based on a simple mixing rule and the temperature dependence of these physical properties is represented by curve fitting equations. These fitting equations can be used for thermal modeling of practical devices/systems at their operation temperatures. The results of the mixing rule showed a consistent correlation between the amount of copper and diamond in the composite, based on density, thermal expansion, and heat capacity measurements. However, there was a disparity between measured and estimated thermal diffusivity and thermal conductivity. These discrepancies can be caused by many intrinsic material issues such as lattice defects and impurities, but the dominant factor is attributed to the large uncertainty of the interfacial thermal conductance between diamond and copper.
Optically induced dynamic nuclear spin polarisation in diamond
Scheuer, Jochen; Schwartz, Ilai; Chen, Qiong; Schulze-Sünninghausen, David; Carl, Patrick; Höfer, Peter; Retzker, Alexander; Sumiya, Hitoshi; Isoya, Junichi; Luy, Burkhard; Plenio, Martin B.; Naydenov, Boris; Jelezko, Fedor
2016-01-01
The sensitivity of magnetic resonance imaging (MRI) depends strongly on nuclear spin polarisation and, motivated by this observation, dynamical nuclear spin polarisation has recently been applied to enhance MRI protocols (Kurhanewicz et al 2011 Neoplasia 13 81). Nuclear spins associated with the 13C carbon isotope (nuclear spin I = 1/2) in diamond possess uniquely long spin lattice relaxation times (Reynhardt and High 2011 Prog. Nucl. Magn. Reson. Spectrosc. 38 37). If they are present in diamond nanocrystals, especially when strongly polarised, they form a promising contrast agent for MRI. Current schemes for achieving nuclear polarisation, however, require cryogenic temperatures. Here we demonstrate an efficient scheme that realises optically induced 13C nuclear spin hyperpolarisation in diamond at room temperature and low ambient magnetic field. Optical pumping of a nitrogen-vacancy centre creates a continuously renewable electron spin polarisation which can be transferred to surrounding 13C nuclear spins. Importantly for future applications we also realise polarisation protocols that are robust against an unknown misalignment between magnetic field and crystal axis.
The evaluation of radiation damage parameter for CVD diamond
Grilj, V., E-mail: vgrilj@irb.hr [Division for Experimental Physics, Ruđer Bošković Institute, 10000 Zagreb (Croatia); Skukan, N.; Jakšić, M. [Division for Experimental Physics, Ruđer Bošković Institute, 10000 Zagreb (Croatia); Pomorski, M. [CEA-LIST, Diamond Sensors Laboratory, Gif-sur-Yvette F-91191 (France); Kada, W. [Division of Electronics and Informatics, Faculty of Science and Technology, Gunma University, Kiryu, Gunma 376-8515 (Japan); Kamiya, T.; Ohshima, T. [Japan Atomic Energy Agency (JAEA), Takasaki, Gunma 370-1292 (Japan)
2016-04-01
There are a few different phenomenological approaches that aim to track the dependence of signal height in irradiated solid state detectors on the fluence of damaging particles. However, none of them are capable to provide a unique radiation hardness parameter that would reflect solely the material capability to withstand high radiation environment. To extract such a parameter for chemical vapor deposited (CVD) diamond, two different diamond detectors were irradiated with proton beams in MeV energy range and subjected afterwards to ion beam induced charge (IBIC) analysis. The change in charge collection efficiency (CCE) due to defects produced was investigated in context of a theoretical model that was developed on the basis of the adjoint method for linearization of the continuity equations of electrons and holes. Detailed modeling of measured data resulted with the first known value of the kσ product for diamond, where k represents the number of charge carriers’ traps created per one simulated primary lattice vacancy and σ represents the charge carriers’ capture cross section. As discussed in the text, this product could be considered as a true radiation damage parameter.
Tailoring exchange couplings in magnetic topological-insulator/antiferromagnet heterostructures
He, Qing Lin; Kou, Xufeng; Grutter, Alexander J.; Yin, Gen; Pan, Lei; Che, Xiaoyu; Liu, Yuxiang; Nie, Tianxiao; Zhang, Bin; Disseler, Steven M.; Kirby, Brian J.; Ratcliff, William, II; Shao, Qiming; Murata, Koichi; Zhu, Xiaodan; Yu, Guoqiang; Fan, Yabin; Montazeri, Mohammad; Han, Xiaodong; Borchers, Julie A.; Wang, Kang L.
2017-01-01
Magnetic topological insulators such as Cr-doped (Bi,Sb)2Te3 provide a platform for the realization of versatile time-reversal symmetry-breaking physics. By constructing heterostructures exhibiting Néel order in an antiferromagnetic CrSb and ferromagnetic order in Cr-doped (Bi,Sb)2Te3, we realize emergent interfacial magnetic phenomena which can be tailored through artificial structural engineering. Through deliberate geometrical design of heterostructures and superlattices, we demonstrate the use of antiferromagnetic exchange coupling in manipulating the magnetic properties of magnetic topological insulators. Proximity effects are shown to induce an interfacial spin texture modulation and establish an effective long-range exchange coupling mediated by antiferromagnetism, which significantly enhances the magnetic ordering temperature in the superlattice. This work provides a new framework on integrating topological insulators with antiferromagnetic materials and unveils new avenues towards dissipationless topological antiferromagnetic spintronics.
Takashi Yanagisawa
2015-01-01
Full Text Available We investigate the ground state of two-dimensional Hubbard model on the basis of the variational Monte Carlo method. We use wave functions that include kinetic correlation and doublon-holon correlation beyond the Gutzwiller ansatz. It is still not clear whether the Hubbard model accounts for high-temperature superconductivity. The antiferromagnetic correlation plays a key role in the study of pairing mechanism because the superconductive phase exists usually close to the antiferromagnetic phase. We investigate the stability of the antiferromagnetic state when holes are doped as a function of the Coulomb repulsion U. We show that the antiferromagnetic correlation is suppressed as U is increased exceeding the bandwidth. High-temperature superconductivity is possible in this region with enhanced antiferromagnetic spin fluctuation and pairing interaction.
Atkinson, D; van Steenwijk, F.J.
The resistance between two arbitrary nodes in an infinite square lattice of:identical resistors is calculated, The method is generalized to infinite triangular and hexagonal lattices in two dimensions, and also to infinite cubic and hypercubic lattices in three and more dimensions. (C) 1999 American
Lattice Regularization and Symmetries
Hasenfratz, Peter; Von Allmen, R; Allmen, Reto von; Hasenfratz, Peter; Niedermayer, Ferenc
2006-01-01
Finding the relation between the symmetry transformations in the continuum and on the lattice might be a nontrivial task as illustrated by the history of chiral symmetry. Lattice actions induced by a renormalization group procedure inherit all symmetries of the continuum theory. We give a general procedure which gives the corresponding symmetry transformations on the lattice.
Are diamond nanoparticles cytotoxic?
Schrand, Amanda M; Huang, Houjin; Carlson, Cataleya; Schlager, John J; Omacr Sawa, Eiji; Hussain, Saber M; Dai, Liming
2007-01-11
Finely divided carbon particles, including charcoal, lampblack, and diamond particles, have been used for ornamental and official tattoos since ancient times. With the recent development in nanoscience and nanotechnology, carbon-based nanomaterials (e.g., fullerenes, nanotubes, nanodiamonds) attract a great deal of interest. Owing to their low chemical reactivity and unique physical properties, nanodiamonds could be useful in a variety of biological applications such as carriers for drugs, genes, or proteins; novel imaging techniques; coatings for implantable materials; and biosensors and biomedical nanorobots. Therefore, it is essential to ascertain the possible hazards of nanodiamonds to humans and other biological systems. We have, for the first time, assessed the cytotoxicity of nanodiamonds ranging in size from 2 to 10 nm. Assays of cell viability such as mitochondrial function (MTT) and luminescent ATP production showed that nanodiamonds were not toxic to a variety of cell types. Furthermore, nanodiamonds did not produce significant reactive oxygen species. Cells can grow on nanodiamond-coated substrates without morphological changes compared to controls. These results suggest that nanodiamonds could be ideal for many biological applications in a diverse range of cell types.
Integrated diamond networks for quantum nanophotonics
Hausmann, Birgit J M; Quan, Qimin; Maletinsky, Patrick; McCutcheon, Murray; Choy, Jennifer T; Babinec, Tom M; Kubanek, Alexander; Yacoby, Amir; Lukin, Mikhail D; Loncar, Marko
2011-01-01
Diamond is a unique material with exceptional physical and chemical properties that offers potential for the realization of high-performance devices with novel functionalities. For example diamond's high refractive index, transparency over wide wavelength range, and large Raman gain are of interest for the implementation of novel photonic devices. Recently, atom-like impurities in diamond emerged as an exceptional system for quantum information processing, quantum sensing and quantum networks. For these and other applications, it is essential to develop an integrated nanophotonic platform based on diamond. Here, we report on the realization of such an integrated diamond photonic platform, diamond on insulator (DOI), consisting of a thin single crystal diamond film on top of an insulating silicon dioxide/silicon substrate. Using this approach, we demonstrate diamond ring resonators that operate in a wide wavelength range, including the visible (630nm) and near-infrared (1,550nm). Finally, we demonstrate an int...
The Design of Diamond Compton Telescope
Hibino, Kinya; Okuno, Shoji; Yajima, Kaori; Uchihori, Yukio; Kitamura, Hisashi; Takashima, Takeshi; Yokota, Mamoru; Yoshida, Kenji
2007-01-01
We have developed radiation detectors using the new synthetic diamonds. The diamond detector has an advantage for observations of "low/medium" energy gamma rays as a Compton telescope. The primary advantage of the diamond detector can reduce the photoelectric effect in the low energy range, which is background noise for tracking of the Compton recoil electron. A concept of the Diamond Compton Telescope (DCT) consists of position sensitive layers of diamond-striped detector and calorimeter layer of CdTe detector. The key part of the DCT is diamond-striped detectors with a higher positional resolution and a wider energy range from 10 keV to 10 MeV. However, the diamond-striped detector is under development. We describe the performance of prototype diamond detector and the design of a possible DCT evaluated by Monte Carlo simulations.
Anodic bonding of diamond to glass
Fuentes, R. [Materials and Technologies Corp., Poughkeepsie, NY (United States); Trolio, L.M. [Geo-Centers, Inc., Fort Washington, MD (United States); Butler, J.E. [Naval Research Lab., Washington, DC (United States)
1995-12-31
A method is described for anodically bonding smooth nanocrystalline diamond films to glass substrates to form extremely flat diamond membranes with the smoothest side available of patterning absorber structures to form masks for proximity focused x-ray lithography.
A new route to process diamond wires
Marcello Filgueira
2003-06-01
Full Text Available We propose an original route to process diamond wires, denominated In Situ Technology, whose fabrication involves mechanical conformation processes, such as rotary forging, copper tubes restacking, and thermal treatments, such as sintering and recrystallisation of a bronze 4 wt.% diamond composite. Tensile tests were performed, reaching an ultimate tensile strength (UTS of 230 MPa for the diameter of Æ = 1.84 mm. Scanning electron microscopy showed the diamond crystals distribution along the composite rope during its manufacture, as well as the diamond adhesion to the bronze matrix. Cutting tests were carried out with the processed wire, showing a probable performance 4 times higher than the diamond sawing discs, however its probable performance was about 5 to 8 times less than the conventional diamond wires (pearl system due to the low abrasion resistance of the bronze matrix, and low adhesion between the pair bronze-diamond due to the use of not metallised diamond single crystals.
Superconductivity in the Kondo lattice model
Bodensiek, Oliver; Pruschke, Thomas [Institute for Theoretical Physics, University of Goettingen, Friedrich-Hund-Platz 1, D-37077 Goettingen (Germany); Zitko, Rok [Institute for Theoretical Physics, University of Goettingen, Friedrich-Hund-Platz 1, D-37077 Goettingen (Germany); Jozef Stefan Institute, Jamova 39, SI-1000 Ljubljana (Slovenia)
2011-07-01
We study the Kondo lattice model with an additional attractive interaction among the conduction-band electrons by means of dynamical mean-field theory in combination with the numerical renormalization group method. In the normal phase we observe a strong dependency of the low-energy scale on the attractive interaction. Thus, there exists a delicate interplay between the attractive interaction and the antiferromagnetic Kondo exchange, which results in a critical interaction, above of which the Fermi surface collapses because the spins become effectively decoupled from the conduction electrons. Additionally, we allow for a s-wave superconducting phase, which appears to be split at the point of the underlying Fermi surface collapse. We discuss the interplay between attractive interaction an Kondo exchange and its pertinence to phonons in heavy fermion physics.
Lattice parameters guide superconductivity in iron-arsenides
Konzen, Lance M. N.; Sefat, Athena S.
2017-03-01
The discovery of superconducting materials has led to their use in technological marvels such as magnetic-field sensors in MRI machines, powerful research magnets, short transmission cables, and high-speed trains. Despite such applications, the uses of superconductors are not widespread because they function much below room-temperature, hence the costly cooling. Since the discovery of Cu- and Fe-based high-temperature superconductors (HTS), much intense effort has tried to explain and understand the superconducting phenomenon. While no exact explanations are given, several trends are reported in relation to the materials basis in magnetism and spin excitations. In fact, most HTS have antiferromagnetic undoped ‘parent’ materials that undergo a superconducting transition upon small chemical substitutions in them. As it is currently unclear which ‘dopants’ can favor superconductivity, this manuscript investigates crystal structure changes upon chemical substitutions, to find clues in lattice parameters for the superconducting occurrence. We review the chemical substitution effects on the crystal lattice of iron-arsenide-based crystals (2008 to present). We note that (a) HTS compounds have nearly tetragonal structures with a-lattice parameter close to 4 Å, and (b) superconductivity can depend strongly on the c-lattice parameter changes with chemical substitution. For example, a decrease in c-lattice parameter is required to induce ‘in-plane’ superconductivity. The review of lattice parameter trends in iron-arsenides presented here should guide synthesis of new materials and provoke theoretical input, giving clues for HTS.
Ohmic contacts to semiconducting diamond
Zeidler, James R.; Taylor, M. J.; Zeisse, Carl R.; Hewett, C. A.; Delahoussaye, Paul R.
1990-10-01
Work was carried out to improve the electron beam evaporation system in order to achieve better deposited films. The basic system is an ion pumped vacuum chamber, with a three-hearth, single-gun e-beam evaporator. Four improvements were made to the system. The system was thoroughly cleaned and new ion pump elements, an e-gun beam adjust unit, and a more accurate crystal monitor were installed. The system now has a base pressure of 3 X 10(exp -9) Torr, and can easily deposit high-melting-temperature metals such as Ta with an accurately controlled thickness. Improved shadow masks were also fabricated for better alignment and control of corner contacts for electrical transport measurements. Appendices include: A Thermally Activated Solid State Reaction Process for Fabricating Ohmic Contacts to Semiconducting Diamond; Tantalum Ohmic Contacts to Diamond by a Solid State Reaction Process; Metallization of Semiconducting Diamond: Mo, Mo/Au, and Mo/Ni/Au; Specific Contact Resistance Measurements of Ohmic Contracts to Diamond; and Electrical Activation of Boron Implanted into Diamond.
Numerical Modeling on Thermal Loading of Diamond Crystal in X-ray FEL Oscillator
Song, Meiqi; Guo, Yuhang; Li, Kai; Deng, Haixiao
2015-01-01
Due to high reflectivity and high resolution to X-ray pulse, diamond is one of the most popular Bragg crystals serving as the reflecting mirror and mono-chromator in the next generation free electrons lasers (FELs). The energy deposition of X-rays will result in thermal heating, and thus lattice expanding of diamond crystal, which may degrade the performance of X-ray FELs. In this paper, the thermal loading effect of diamond crystal for X-ray FEL oscillator has been systematically studied by the combined simulation of Geant4 and ANSYS, and its dependence on the environment temperature, crystal size, X-ray pulse repetition rate and pulse energy are presented.
SAJAD HUSSAIN DIN; M A SHAH; N A SHEIKH; K A NAJAR; K RAMASUBRAMANIAN; S BALAJI; M S RAMACHANDRA RAO
2016-12-01
Titanium alloy (Ti6Al4V) substrates were deposited with smooth multilayer coatings, by hot filament chemical vapour deposition technique. The effect of boron doping on lattice parameter, residual stresses, hardness and coefficient of friction in multilayer-diamond coating system was studied. The frictional behaviour of the coatings was studied using a ball-on-disc micro-tribometer by sliding the coated samples of titanium alloy (Ti6Al4V) substrates against alumina (Al$_2$O$_3$) balls, and increasing normal load from 1 to 10N. The average friction coefficient decreased from 0.36 to 0.29 for undoped multilayer-diamond coating system and from 0.33 to 0.18 for borondoped (BD) multilayer-diamond coating system. The average indentation depths for undoped and BD multilayerdiamond coating systems were found to be equal to $\\sim$58 and $\\sim$65 nm, respectively, and their hardness values were 60 and 55~GPa, respectively.
Shurter, R.P.; Moir, D.C.; Devlin, D.J.; Springer, R.W.
1997-08-01
Investigations are underway at Los Alamos to develop a new generation of high current, low source temperature photo cathodes able to operate in vacuum environments with pressures above 10e-6 torr without poisoning or degradation of emission properties. Polycrystalline diamond films are emerging as the ideal material for these photocathodes. Robustness, high quantum efficiency and high thermal conductivity are fundamental necessary attributes that are found in diamond. The high electron/hole mobility in the boron doped diamond lattice and the ability to create a negative electron affinity surface through downward band bending allow for high current density emission with quantum efficiencies of 0.5% when illuminated by a ArF laser. We report the results to date toward the development of a four kiloampere photocathode with a source temperature below 5eV for the DARHT linear induction Accelerator
Gofryk, K. [Idaho National Lab. (INL), Idaho Falls, ID (United States); Jaime, M. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States). National High Magnetic Field Lab. (MagLab)
2014-12-01
Our preliminary magnetostriction measurements have already shown a strong interplay of lattice dynamic and magnetism in both antiferromagnetic and paramagnetic states, and give unambiguous evidence of strong spin- phonon coupling in uranium dioxide. Further studies are planned to address the puzzling behavior of UO_{2} in magnetic and paramagnetic states and details of the spin-phonon coupling.
Development of Diamond-Coated Drills
无
2002-01-01
Compared with the sintered polycrystalline diamond, the deposited thin film diamond has the great advantage on the fabrication of cutting tools with complex geometries such as drills. Because of their low costs for fabrication equipment and high performance on high speed machining non-ferrous metals and alloys, metal-compound materials, and hard brittle non-metals, diamond-coated drills find great potentialities in the commercial application. However, the poor adhesion of the diamond film on the substrate...
Raman spectral research on MPCVD diamond film
YAN Yan; ZHANG Shulin; ZHAO Xinsheng; HAN Yisong; HOU Li
2003-01-01
Raman spectra of MPCVD diamond film have been studied. Based on the resonance size selection effect, we think that there is no nano-crystalline diamond in the sample and the Raman peak at 1145 cm-1 can not be considered as the characteristic peak of nano-crystalline diamond though it has been used as the characteristic peak of nano-crystalline diamond widely for many years.
Medical applications of diamond particles & surfaces
Roger J Narayan
2011-04-01
Full Text Available Diamond has been considered for use in several medical applications due to its unique mechanical, chemical, optical, and biological properties. In this paper, methods for preparing synthetic diamond surfaces and particles are described. In addition, recent developments involving the use of diamond in prostheses, sensing, imaging, and drug delivery applications are reviewed. These developments suggest that diamond-containing structures will provide significant improvements in the diagnosis and treatment of medical conditions over the coming years.
Diamond and diamond-like films for transportation applications
Perez, J.M.
1993-01-01
This section is a compilation of transparency templates which describe the goals of the Office of Transportation Materials (OTM) Tribology Program. The positions of personnel on the OTM are listed. The role and mission of the OTM is reviewed. The purpose of the Tribology Program is stated to be `to obtain industry input on program(s) in tribology/advanced lubricants areas of interest`. The objective addressed here is to identify opportunities for cost effective application of diamond and diamond-like carbon in transportation systems.
Kolawa, Elizabeth A. (Inventor); Patel, Jagdishbhai U. (Inventor); Fleurial, Jean-Pierre (Inventor)
2004-01-01
A power source that converts a-particle energy into electricity by coulomb collision in doped diamond films is described. Alpha particle decay from curium-244 creates electron-hole pairs by free- ing electrons and holes inside the crystal lattice in N- and P-doped diamond films. Ohmic contacts provide electrical connection to an electronic device. Due to the built-in electric field at the rectifying junction across the hT- and P-doped diamond films, the free electrons are constrained to traveling in generally one direction. This one direction then supplies electrons in a manner similar to that of a battery. The radioactive curium layer may be disposed on diamond films for even distribution of a-particle radiation. The resulting power source may be mounted on a diamond substrate that serves to insulate structures below the diamond substrate from a-particle emission. Additional insulation or isolation may be provided in order to prevent damage from a-particle collision. N-doped silicon may be used instead of N-doped diamond.
Zhang, Yu-Jun; Chen, Jia-Hui; Li, Liang-Liang; Ma, Jing; Nan, Ce-Wen; Lin, Yuan-Hua
2017-05-01
Electric field manipulation of magnetic properties has attracted a lot of research interest recently in solid-state physics. However, ferroelectric strain modulation of antiferromagnetic (AFM) layer is rarely studied in ferromagnet/antiferromagnet/ferroelectric heterostructures. In this paper, we prepared a Ni/NiO(001) heterostructure on ferroelectric Pb (Mg1/3N b2 /3 ) 0.7T i0.3O3(001 ) substrates and observed an out-of-plane electric field modulation of exchange bias and magnetic anisotropy in the Ni layer. The exchange bias was easily eliminated by an electric field cycle, which was due to the AFM domain switching induced by piezoelectric strain in the NiO layer. Synchrotron x ray linear dichroism results confirmed the AFM moment alignment induced by ferroelectric strain as well. Our work showed a promising strategy to manipulate AFM moments and domains, serving the blooming AFM spintronics.
Maeter, H; Zvyagin, A A; Luetkens, H; Pascua, G; Shermadini, Z; Saint-Martin, R; Revcolevschi, A; Hess, C; Büchner, B; Klauss, H-H
2013-09-11
We report zero and longitudinal magnetic field muon spin relaxation (μSR) measurements of the spin S = 1/2 antiferromagnetic Heisenberg chain material SrCuO2. We find that in a weak applied magnetic field B0 the spin-lattice relaxation rate λ follows a power law λ is proportional to B(0)(-n) with n = 0.9(3). This result is temperature independent for 5 K ≤ T ≤ 300 K. Within conformal field theory and using the Müller ansatz we conclude ballistic spin transport in SrCuO2.
Sousa, Griffith Mendonça A., E-mail: griffith_mas@hotmail.com; Pires, A.S.T.
2014-03-15
The Neel and collinear ordered phases of the two-dimensional S=1 antiferromagnet with next and next near neighbor exchange interactions and easy axis single ion anisotropy, on the square lattice, are studied at low temperature using a Modified Spin Wave Theory. We calculate the low-temperature quantities as a function of the temperature, frustration and anisotropy. We calculate also the phase diagram at T=0. We found a disordered phase separating the Neel and collinear phases. - Highlights: • The phase diagrams in zero temperature. • The critical temperature was studied as a function of frustration and D. • The sublattice magnetizations and the gap were studied.
Diamond Drilling Specification Manual and Course Outline.
British Columbia Dept. of Education, Victoria.
This publication presents the standards required of a person practicing diamond drilling in western Canada and provides an outline for teaching the skills and knowledge. It is divided into two parts. The Diamond Drilling Specification Manual establishes the levels of skill and knowledge required in the four certified levels of diamond drilling.…
Ultratough single crystal boron-doped diamond
Hemley, Russell J [Carnegie Inst. for Science, Washington, DC ; Mao, Ho-Kwang [Carnegie Inst. for Science, Washington, DC ; Yan, Chih-Shiue [Carnegie Inst. for Science, Washington, DC ; Liang, Qi [Carnegie Inst. for Science, Washington, DC
2015-05-05
The invention relates to a single crystal boron doped CVD diamond that has a toughness of at least about 22 MPa m.sup.1/2. The invention further relates to a method of manufacturing single crystal boron doped CVD diamond. The growth rate of the diamond can be from about 20-100 .mu.m/h.
Katarina Anthony
2015-01-01
Alongside the CMS Pixel Luminosity Telescope (PLT) – installed last month (see here) – lie diamond detectors. No ordinary gems, these lab-grown diamonds will be playing a vital role in Run 2: differentiating signals from collision products with those from the beam background. The BCM detector's green "c-shaped" printed circuit board is mounted on the PLT/BCM carbon-fibre carriage ready for installation. Earlier this year, the CMS BRIL project installed beam condition monitors (BCM) at the heart of the CMS detector. Designed to measure the online luminosity and beam background as close as possible to the LHC beam pipe, the BCMs use radiation-hard diamonds to differentiate between background and collision signals. The BCM also protects the CMS silicon trackers from damaging beam losses, by aborting the beam if the signal currents measured are above an acceptable threshold. These new BCMs are designed with Run 2 bunches in mind. &ldq...
Fractal dimension in percolating Heisenberg antiferromagnets
Itoh, S. [Neutron Science Laboratory, High Energy Accelerator Research Organization, Tsukuba 305-0810 (Japan)]. E-mail: shinichi.itoh@kek.jp; Kajimoto, R. [Quantum Beam Science Directorate, Japan Atomic Energy Agency, Tokai 319-1195 (Japan); Adams, M.A. [ISIS Facility, Rutherford Appleton Laboratory, Didcot, Oxon OX11 0QX (United Kingdom); Bull, M.J. [ISIS Facility, Rutherford Appleton Laboratory, Didcot, Oxon OX11 0QX (United Kingdom); Iwasa, K. [Department of Physics, Tohoku University, Sendai 980-8578 (Japan); Aso, N. [Neutron Science Laboratory, Institute for Solid State Physics, University of Tokyo, Tokai 319-1106 (Japan); Yoshizawa, H. [Neutron Science Laboratory, Institute for Solid State Physics, University of Tokyo, Tokai 319-1106 (Japan); Takeuchi, T. [Low Temperature Center, Osaka University, Toyonaka 560-0043 (Japan)
2007-03-15
We investigated static and dynamical properties in the three-dimensional percolating Heisenberg antiferromagnets, RbMn{sub c}Mg{sub 1-c}F{sub 3}, with the magnetic concentration close to the percolation threshold, c{sub P}=0.312, around the superlattice point well below T{sub N}. In neutron diffraction experiment, the wave number dependence of the elastic scattering component was well fitted to q{sup -x}. Magnetic fractons were also studied using inelastic neutron scattering, and the observed fractons showed the dispersion relation of q{sup z}. The determined exponents, x=2.43+/-0.05 and z=2.5+/-0.1, were in good agreement with the fractal dimension (D{sub f}=2.48)
Magnetic Properties of Nanoparticles of Antiferromagnetic Materials
Mørup, Steen; Frandsen, Cathrine; Bødker, Franz
2003-01-01
The magnetic properties of antiferromagnetic nanoparticles have been studied by Mossbauer spectroscopy and neutron scattering. Temperature series of Mossbauer spectra of non-interacting, superparamagnetic hematite nanoparticles were fitted by use of the Blume-Tjon relaxation model. It has been...... found that the magnetic anisotropy energy constant increases significantly with decreasing particle size. Neutron scattering experiments on similar samples give new information on both superparamagnetic relaxation and collective magnetic excitations. There is good agreement between the values...... of the parameters obtained from Mossbauer spectroscopy and neutron scattering. In samples of interacting hematite nanoparticles, the relaxation was significantly suppressed. The Mossbauer data for these samples are in accordance with a mean field model for an ordered state of strongly interacting particles. Mixing...
Antiferromagnetic spin wave and the superconductivity
Koh, Shun-ichiro
2000-07-01
The neutron scattering of UPd 2Al 3 showed that a sharp peak, which is absent in the normal phase, appears in the superconducting phase (Metoki et al., J. Phys. Soc. Japan 66 (1997) 2560; Bernhoeft et al., Phys. Rev. Lett. 81 (1998) 4244). Assuming this excitation to be an antiferromagnetic (AFM) spin-wave, this paper deals with its enhancement by the superconductivity. Applying the slave-boson formalism, we consider the AFM ordering as a spin-density-wave (Koh, Phys. Lett. A 253 (1999) 98). Above Tc, the spin-wave suffers an energy dissipation due to the conduction electron. Below Tc, the superconductivity suppresses the dissipation, resulting in the growth of the AFM spin-wave.
Spin dynamics in geometrically frustrated antiferromagnetic pyrochlores
Gardner, J. S.; Ehlers, G.; Bramwell, S. T.; Gaulin, B. D.
2004-03-01
We have studied the spin dynamics of several antiferromagnetic pyrochlore oxides. These magnets are geometrically frustrated and only reach their ground states at temperatures much lower than that expected from mean field theory. Here we present data on the magnetic nature, especially the spin dynamics of Tb2Ti2O7, Gd2Ti2O7 and Y2Mo2O7. In these systems the ground states are found to be very different. Y2Mo2O7 freezes completely into a spin glass-like state, Tb2Ti2O7 is a cooperative paramagnetic and remains dynamic down to 15 mK and Gd2Ti2O7 enters a unique partially ordered state at {\\sim }1 K.
Pulsed laser deposition of metallic films on the surface of diamond particles for diamond saw blades
Jiang Chao [State Key Laboratory of Laser Technology, Huazhong University of Science and Technology, WuHan, Hubei 430074 (China); Luo Fei [State Key Laboratory of Laser Technology, Huazhong University of Science and Technology, WuHan, HuBei 430074 (China); Long Hua [State Key Laboratory of Laser Technology, Huazhong University of Science and Technology, Wuhan, Hubei 430074 (China); Hu Shaoliu [State Key Laboratory of Laser Technology, Huazhong University of Science and Technology, Wuhan, Hubei 430074 (China); Li Bo [State Key Laboratory of Laser Technology, Huazhong University of Science and Technology, Wuhan, Hubei 430074 (China); Wang Youqing [State Key Laboratory of Laser Technology, Huazhong University of Science and Technology, Wuhan, Hubei 430074 (China)]. E-mail: lchwan@hust.edu.cn
2005-06-15
Ti or Ni films have been deposited on the diamond particle surfaces by pulsed laser deposition. Compressive resistance of the uncoated and coated diamond particles was measured, respectively, in the experiments. The compressive resistance of the Ti-coated diamonds particles was found much higher than that of the uncoated ones. It increased by 39%. The surface morphology is observed by the metallography microscope. The surface of the uncoated diamonds particles had many hollows and flaws, while the surface of Ni-coated diamond particles was flat and smooth, and the surface of Ti-coated diamond particles had some metal masses that stood out of the surface of the Ti-coated film. The components of the metallic films of diamond particles were examined by X-ray diffractometry (XRD). TiC was found formed on the Ti-coated diamond surface, which resulted in increased surface bonding strength between the diamond particles and the Ti films. Meanwhile, TiC also favored improving the bonding strength between the coated diamond particles and the binding materials. Moreover, the bending resistance of the diamond saw blade made of Ti-coated diamond was drastically higher than that of other diamond saw blades, which also played an important role in improving the blade's cutting ability and lifetime. Therefore, it was most appropriate that the diamond saw blade was made of Ti-coated diamond particles rather than other materials.
Quasiparticle bandstructure of antiferromagnetic EuTe
Mathi Jaya, S.; Nolting, W.
1997-11-01
The temperature-dependent electronic quasiparticle spectrum of the antiferromagnetic semiconductor EuTe is derived by use of a combination of a many-body model procedure with a tight-binding - `linear muffin tin orbital' (TB - LMTO) band structure calculation. The central part is the d - f model for a single band electron (`test electron') being exchange coupled to the antiferromagnetically ordered localized moments of the Eu ions. The single-electron Bloch energies of the d - f model are taken from a TB - LMTO calculation for paramagnetic EuTe. The d - f model is evaluated by a recently proposed moment conserving Green function technique to get the temperature-dependent sublattice - quasiparticle bandstructure (S - QBS) and sublattice - quasiparticle density of states (S - QDOS) of the unoccupied 5d - 6s energy bands. Unconventional correlation effects and the appearance of characteristic quasiparticles (`magnetic polarons') are worked out in detail. The temperature dependence of the S - QDOS and S - QBS is mainly provoked by the spectral weights of the energy dispersions. Minority- and majority-spin spectra coincide for all temperatures but with different densities of states. Upon cooling from 0953-8984/9/47/012/img1 to T = 0 K the lower conduction band edge exhibits a small blue shift of -0.025 eV in accordance with the experiment. Quasiparticle damping manifesting itself in a temperature-dependent broadening of the spectral density peaks arises from spin exchange processes between (5d - 6s) conduction band electrons and localized 4f moments.
Diamonds on Diamond: structural studies at extreme conditions on the Diamond Light Source.
McMahon, M I
2015-03-06
Extreme conditions (EC) research investigates how the structures and physical and chemical properties of materials change when subjected to extremes of pressure and temperature. Pressures in excess of one million times atmospheric pressure can be achieved using a diamond anvil cell, and, in combination with high-energy, micro-focused radiation from a third-generation synchrotron such as Diamond, detailed structural information can be obtained using either powder or single-crystal diffraction techniques. Here, I summarize some of the research drivers behind international EC research, and then briefly describe the techniques by which high-quality diffraction data are obtained. I then highlight the breadth of EC research possible on Diamond by summarizing four examples from work conducted on the I15 and I19 beamlines, including a study which resulted in the first research paper from Diamond. Finally, I look to the future, and speculate as to the type of EC research might be conducted at Diamond over the next 10 years.
Electrically tunable transport in antiferromagnetic Sr3Ir2O7
Seinige, Heidi; Wang, Cheng; Cao, Gang; Zhou, Jianshi-S.; Goodenough, John B.; Tsoi, Maxim
Recently we demonstrated experimentally the existence of interconnections between magnetic state and transport currents in antiferromagnetic (AFM) Mott insulator Sr2IrO4. We found a very large anisotropic magnetoresistance and demonstrated a reversible resistive switching driven by high-density currents/high electric fields. These results support the feasibility of AFM spintronics, where antiferromagnets are used in place of ferromagnets, however a low Néel temperature of this material (240 K) questions any practical applications. Here we present a comparative electrical transport study of its sister compound Sr2IrO4 which has a higher transition temperature (285 K). Similar to the case of Sr2IrO4, we find a continuous reduction in the resistivity of Sr3Ir2O7 as a function of increasing electrical bias and abrupt reversible changes above a threshold bias current. We explain these results by a reduction of activation energy associated with a field-driven lattice distortion. This work was supported in part by C-SPIN, one of six centers of STARnet, a Semiconductor Research Corporation program, sponsored by MARCO and DARPA, and by NSF Grants DMR-1207577, DMR-1265162, and DMR-1122603.
Excitation-Gap Scaling near Quantum Critical Three-Dimensional Antiferromagnets.
Lohöfer, M; Wessel, S
2017-04-07
By means of large-scale quantum Monte Carlo simulations, we examine the quantum critical scaling of the magnetic excitation gap (the triplon gap) in a three-dimensional dimerized quantum antiferromagnet, the bicubic lattice, and identify characteristic multiplicative logarithmic scaling corrections atop the leading mean-field behavior. These findings are in accord with field-theoretical predictions that are based on an effective description of the quantum critical system in terms of an asymptotically free field theory, which exhibits a logarithmic decay of the renormalized interaction strength upon approaching the quantum critical point. Furthermore, using bond-based singlet spectroscopy, we identify the amplitude (Higgs) mode resonance within the antiferromagnetic region. We find a Higgs mass scaling in accord with field-theoretical predictions that relate it by a factor of sqrt[2] to the corresponding triplon gap in the quantum disordered regime. In contrast to the situation in lower-dimensional systems, we observe in this three-dimensional coupled-dimer system a distinct signal from the amplitude mode also in the dynamical spin structure factor. Its width is observed to vanish proportional to the Higgs mass in the accessible proximity to the quantum critical point.
Strongly Coupled Systems: From Quantum Antiferromagnets To Unified Models For Superconductors
Chudnovsky, V
2002-01-01
I discuss the significance of the antiferromagnetic Heisenberg model (AFHM) in both high-energy and condensed-matter physics, and proceed to describe an efficient cluster algorithm used to simulate the AFHM. This is one of two algorithms with which my collaborators and I were able to obtain numerical results that definitively confirm that chiral perturbation theory, corrected for cutoff effects in the AFHM, leads to a correct field-theoretical description of the low- temperature behavior of the spin correlation length in various spin representations S. Using a finite-size-scaling technique, we explored correlation lengths of up to 105 lattice spacings for spins S = 1 and 5/2. We show how the recent prediction of cutoff effects by P. Hasenfratz is approached for moderate correlation lengths, and smoothly connects with other approaches to modeling the AFHM at smaller correlation lengths. I also simulate and discuss classical antiferromagnetic systems with simultaneous SO(M) and SO( N) symmetries, which have bee...
Strongly Coupled Systems From Quantum Antiferromagnets To Unified Models For Superconductors
Chudnovsky, V
2002-01-01
I discuss the significance of the antiferromagnetic Heisenberg model (AFHM) in both high-energy and condensed-matter physics, and proceed to describe an efficient cluster algorithm used to simulate the AFHM. This is one of two algorithms with which my collaborators and I were able to obtain numerical results that definitively confirm that chiral perturbation theory, corrected for cutoff effects in the AFHM, leads to a correct field-theoretical description of the low- temperature behavior of the spin correlation length in various spin representations S. Using a finite-size-scaling technique, we explored correlation lengths of up to 105 lattice spacings for spins S = 1 and 5/2. We show how the recent prediction of cutoff effects by P. Hasenfratz is approached for moderate correlation lengths, and smoothly connects with other approaches to modeling the AFHM at smaller correlation lengths. I also simulate and discuss classical antiferromagnetic systems with simultaneous SO(M) and SO( N) symmetries, which have bee...
Frustrated antiferromagnet YbAgGe under magnetic fields and pressures
Kubo, Hirokazu; Umeo, Kazunori; Takabatake, Toshiro [ADSM, Hiroshima University, Higashi-Hiroshima 739-8530 (Japan); Katoh, Kenichi [Department of Applied Physics, National Defense Academy, Yokosuka 239-8686 (Japan); Ochiai, Akira, E-mail: khirokazu@hiroshima-u.ac.j [Department of Physics, Graduate School of Science, Tohoku University, Sendai 980-8578 (Japan)
2010-01-15
We present a detailed study of the field (B)- temperature (T) phase diagram under pressures (P) up to 2.7 GPa for the heavy-fermion antiferromagnet YbAgGe that crystallizes in the hexagonal ZrNiAl-type structure with a quasi-kagome lattice of Yb ions. This compound undergoes two magnetic transitions at T{sub M1} = 0.8 K and T{sub M2} = 0.65 K in zero field at ambient pressure. In the ground state, M(B) shows a metamagnetic transition at B{sub M} = 4.6 T for the easy magnetization direction B || a. This transition field decreases to 3.3 T as P is increased to 2.2 GPa. At 2.7 GPa, {rho}(B) exhibits successive transitions at 5.0, 6.0, 7.5, and 9.0 T. On the other hand, for the hard direction B || c, T{sub M} increases with applied field in the P range above 0.5 GPa. This increase of T{sub M}(B) is opposite to the decrease of T{sub M}(B) for a conventional antiferromagnetic phase. These findings suggest that the application of pressure releases in part the magnetic frustration in YbAgGe.
Critical Space-Time Networks and Geometric Phase Transitions from Frustrated Edge Antiferromagnetism
Trugenberger, Carlo A
2015-01-01
Recently I proposed a simple dynamical network model for discrete space-time which self-organizes as a graph with Hausdorff dimension d_H=4. The model has a geometric quantum phase transition with disorder parameter (d_H-d_s) where d_s is the spectral dimension of the dynamical graph. Self-organization in this network model is based on a competition between a ferromagnetic Ising model for vertices and an antiferromagnetic Ising model for edges. In this paper I solve a toy version of this model defined on a bipartite graph in the mean field approximation. I show that the geometric phase transition corresponds exactly to the antiferromagnetic transition for edges, the dimensional disorder parameter of the former being mapped to the staggered magnetization order parameter of the latter. The model has a critical point with long-range correlations between edges, where a continuum random geometry can be defined, exactly as in Kazakov's famed 2D random lattice Ising model but now in any number of dimensions.
Anisotropic spin model of strong spin-orbit-coupled triangular antiferromagnets
Li, Yao-Dong; Wang, Xiaoqun; Chen, Gang
2016-07-01
Motivated by the recent experimental progress on the strong spin-orbit-coupled rare-earth triangular antiferromagnet, we analyze the highly anisotropic spin model that describes the interaction between the spin-orbit-entangled Kramers' doublet local moments on the triangular lattice. We apply the Luttinger-Tisza method, the classical Monte Carlo simulation, and the self-consistent spin wave theory to analyze the anisotropic spin Hamiltonian. The classical phase diagram includes the 120∘ state and two distinct stripe-ordered phases. The frustration is very strong and significantly suppresses the ordering temperature in the regimes close to the phase boundary between two ordered phases. Going beyond the semiclassical analysis, we include the quantum fluctuations of the spin moments within a self-consistent Dyson-Maleev spin-wave treatment. We find that the strong quantum fluctuations melt the magnetic order in the frustrated regions. We explore the magnetic excitations in the three different ordered phases as well as in strong magnetic fields. Our results provide a guidance for the future theoretical study of the generic model and are broadly relevant for strong spin-orbit-coupled triangular antiferromagnets such as YbMgGaO4, RCd3P3 , RZn3P3 , RCd3As3 , RZn3As3 , and R2O2CO3 .
Crucial role of interlayer distance for antiferromagnet-induced perpendicular magnetic anisotropy
Wang, Bo-Yao; Lin, Po-Han; Tsai, Ming-Shian; Shih, Chun-Wei; Lee, Meng-Ju; Huang, Chun-Wei; Jih, Nae-Yeou; Cheng, Pei-Yu; Wei, Der-Hsin
2015-12-01
Antiferromagnetic (AFM) thin films were recently proposed to be an alternative to conventional materials for achieving perpendicular magnetic anisotropy (PMA) in ferromagnetic thin films, because AFM thin films exhibit an advantage of flexible control. Here, we report that antiferromagnet-induced PMA is highly sensitive to interfacial moments of AFM thin films as well as the magnetic interaction of such moments with volume moments, determined according to the vertical interlayer distance. Magnetic hysteresis loops and x-ray magnetic domain imaging revealed the establishment of perpendicular magnetization on face-centered tetragonal (fct)-like Mn/Co/Ni films when covered with monolayered Mn films. A cover of Mn films that exhibit contracted fct- [vertical-to-in-plane lattice constant ratio (c /a )=0.95 ] and expanded fct-like (c /a =1.05 ) structures at different thickness levels induced in-plane magnetic anisotropy and PMA in Co/Ni films, respectively, confirming that the interlayer distance is a crucial parameter for establishing perpendicular magnetization.
Zakhidov, A. A.; Baughman, R. H.; Iqbal, Z.; Khayrullin, I. I.; Ralchenko, V. G.
1998-03-01
We demonstrate a new method for the formation of photonic bandgap crystals that operate at optical wavelengths. This method involves the templating of a self-assempled SiO2 lattice with diamond, graphite, or amorphous forms of carbon, followed by the removal of the original SiO2 lattice matrix by chemical means. Such carbon opal replicas are the "air type" of photonic crystal (where air replaces silica spheres) that are most favourable for photonic bandgap formation. Surprisingly, the structure of the original opal lattice having a typical cubic lattice dimension of 250 nm) is reliably replicated down to the nanometer scale using either a diamond, graphite, or amorphous carbon templated material. The optical properties of these photonic bandgap crystals are reported and compared with both theory and experimental results on other types of opal-derived lattices that we have investigated. The graphitic reverse opal is the first example of a network type metallic photonic crystal for the optical domain, for which a large photonic bandgap have been predicted.
Julia sets and complex singularities in diamond-like hierarchical Potts models
QIAO; Jianyong
2005-01-01
We study the phase transition of the Potts model on diamond-like hierarchical lattices. It is shown that the set of the complex singularities is the Julia set of a rational mapping. An interesting problem is how are these singularities continued to the complex plane. In this paper, by the method of complex dynamics, we give a complete description about the connectivity of the set of the complex singularities.
Ohta, N; Niki, T; Kirihara, S, E-mail: n-ohta@jwri.osaka-u.ac.jp [Smart Processing Research Center, Joining and Welding Research Institute, Osaka University, Ibaraki, Osaka, 567-0047 (Japan)
2011-05-15
Terahertz wave resonators composed of alumina photonic crystals with diamond lattice structures were designed and fabricated by using micro stereolithography. These three dimensional periodic structures can reflect perfectly electromagnetic waves through Bragg diffraction. A micro glass cell including water solutions was put between the photonic crystals as a novel resonance sensor with terahertz frequency range. The localized and amplified waves in the resonators were measured by a spectroscopy, and visualized by theoretical simulations.
Chiral Spin Liquid on a Kagome Antiferromagnet Induced by the Dzyaloshinskii-Moriya Interaction
Messio, Laura; Bieri, Samuel; Lhuillier, Claire; Bernu, Bernard
2017-06-01
The quantum spin liquid material herbertsmithite is described by an antiferromagnetic Heisenberg model on the kagome lattice with a non-negligible Dzyaloshinskii-Moriya interaction (DMI). A well-established phase transition to the q =0 long-range order occurs in this model when the DMI strength increases, but the precise nature of a small-DMI phase remains controversial. Here, we describe a new phase obtained from Schwinger-boson mean-field theory that is stable at small DMI, and which can explain the dispersionless spectrum seen in the inelastic neutron scattering experiment by Han et al. [Nature (London) 492, 406 (2012), 10.1038/nature11659]. It is a time-reversal symmetry breaking Z2 spin liquid, with the unique property of a small and constant spin gap in an extended region of the Brillouin zone. The phase diagram as a function of DMI and spin size is given, and dynamical spin structure factors are presented.
Anomalous curie response of impurities in quantum-critical spin-1/2 Heisenberg antiferromagnets.
Höglund, Kaj H; Sandvik, Anders W
2007-07-13
We consider a magnetic impurity in two different S=1/2 Heisenberg bilayer antiferromagnets at their respective critical interlayer couplings separating Néel and disordered ground states. We calculate the impurity susceptibility using a quantum Monte Carlo method. With intralayer couplings in only one of the layers (Kondo lattice), we observe an anomalous Curie constant C*, as predicted on the basis of field-theoretical work [S. Sachdev, Science 286, 2479 (1999)10.1126/science.286.5449.2479]. The value C* = 0.262 +/- 0.002 is larger than the normal Curie constant C=S(S+1)/3. Our low-temperature results for a symmetric bilayer are consistent with a universal C*.
Theoretical reconsideration of antiferromagnetic Fermi surfaces in URu{sub 2}Si{sub 2}
Yamagami, Hiroshi, E-mail: yamagami@cc.kyoto-su.ac.jp [Department of Physics, Faculty of Science, Kyoto Sangyo University, Kyoto 603-8555 (Japan)
2011-01-01
In an itinerant 5f-band model, the antiferromagnetic (AFM) Fermi surfaces of URu{sub 2}Si{sub 2} are reconsidered using a relativistic LAPW method within a local spin-density approximation, especially taking into account the lattice parameters dependent on pressures. The reduction of the z-coordinate of the Si sites results in the effect of flattening the Ru-Si layers of URu{sub 2}Si{sub 2} crystal structure, thus weakening a hybridization/mixing between the U-5f and Ru-4d states in the band structure. Consequently the 5f bands around the Fermi level are more flat in the dispersion with decreasing the z-coordinate, thus producing three closed Fermi surfaces like 'curing-stone', 'rugby-ball' and 'ball'. The origins of de Haas-van Alphen branches can be qualitatively interpreted from the obtained AFM Fermi surfaces.
Nishimoto, Satoshi; Shibata, Naokazu; Hotta, Chisa
2013-01-01
Quantum spin-1/2 kagome Heisenberg antiferromagnet is the representative frustrated system possibly hosting a spin liquid. Clarifying the nature of this elusive topological phase is a key challenge in condensed matter; however, even identifying it still remains unsettled. Here we apply a magnetic field and discover a series of spin-gapped phases appearing at five different fractions of magnetization by means of a grand canonical density matrix renormalization group, an unbiased state-of-the-art numerical technique. The magnetic field dopes magnons and first gives rise to a possible Z₃ spin liquid plateau at 1/9 magnetization. Higher field induces a self-organized super-lattice unit, a six-membered ring of quantum spins, resembling an atomic orbital structure. Putting magnons into this unit one by one yields three quantum solid plateaus. We thus find that the magnetic field could control the transition between various emergent phases by continuously releasing the frustration.
Magnetic phase diagram of the antiferromagnetic pyrochlore Gd2 Ti2 O7
Petrenko, O. A.; Lees, M. R.; Balakrishnan, G.; Paul, D. Mck
2004-07-01
Gd2Ti2O7 is a highly frustrated antiferromagnet on a pyrochlore lattice, where apart from the Heisenberg exchange the spins also interact via dipole-dipole forces. We report on low-temperature specific heat measurements performed on single crystals of Gd2Ti2O7 for three different directions of an applied magnetic field. The measurements reveal the strongly anisotropic behavior of Gd2Ti2O7 in a magnetic field despite the apparent absence of a significant single-ion anisotropy for Gd3+ . The H-T phase diagrams are constructed for H∥[111] , H∥[110] , and H∥[112] . The results indicate that further theoretical work beyond a simple mean-field model is required.
Solitary Magnons in the S =5/2 Antiferromagnet CaFe2O4
Stock, C.; Rodriguez, E. E.; Lee, N.; Green, M. A.; Demmel, F.; Ewings, R. A.; Fouquet, P.; Laver, M.; Niedermayer, Ch.; Su, Y.; Nemkovski, K.; Rodriguez-Rivera, J. A.; Cheong, S.-W.
2016-07-01
CaFe2O4 is a S =5/2 anisotropic antiferromagnet based upon zig-zag chains having two competing magnetic structures, denoted as the A (↑↑↓↓) and B (↑↓↑↓) phases, which differ by the c -axis stacking of ferromagnetic stripes. We apply neutron scattering to demonstrate that the competing A and B phase order parameters result in magnetic antiphase boundaries along c which freeze on the time scale of ˜1 ns at the onset of magnetic order at 200 K. Using high resolution neutron spectroscopy, we find quantized spin wave levels and measure 9 such excitations localized in regions ˜1 - 2 c -axis lattice constants in size. We discuss these in the context of solitary magnons predicted to exist in anisotropic systems. The magnetic anisotropy affords both competing A +B orders as well as localization of spin excitations in a classical magnet.
Revealing hidden antiferromagnetic correlations in doped Hubbard chains via string correlators
Hilker, Timon A.; Salomon, Guillaume; Grusdt, Fabian; Omran, Ahmed; Boll, Martin; Demler, Eugene; Bloch, Immanuel; Gross, Christian
2017-08-01
Topological phases, like the Haldane phase in spin-1 chains, defy characterization through local order parameters. Instead, nonlocal string order parameters can be employed to reveal their hidden order. Similar diluted magnetic correlations appear in doped one-dimensional lattice systems owing to the phenomenon of spin-charge separation. Here we report on the direct observation of such hidden magnetic correlations via quantum gas microscopy of hole-doped ultracold Fermi-Hubbard chains. The measurement of nonlocal spin-density correlation functions reveals a hidden finite-range antiferromagnetic order, a direct consequence of spin-charge separation. Our technique, which measures nonlocal order directly, can be readily extended to higher dimensions to study the complex interplay between magnetic order and density fluctuations.
Fermi surface evolution and checker-board block-spin antiferromagnetism in AxFe2-ySe2
Tai, Yuan-Yen; Zhu, Jian-Xin; Graf, Matthias J.; Ting, C. S.
2012-10-01
We develop an effective multiorbital mean-field t-J Hamiltonian with realistic tight-binding and exchange parameters to describe the electronic and magnetic structures of iron-selenide based superconductors AxFe2-ySe2 for iron vacancy doping in the range 0≤y≤0.4. The Fermi surface topology extracted from the spectral function of angle-resolved photoemission spectroscopy (ARPES) experiments is adequately accounted for by a tight-binding lattice model with random vacancy disorder. Since introducing iron vacancies breaks the lattice periodicity of the stochiometric compound, it greatly affects the electronic band structure. With changing vacancy concentration, the electronic band structure evolves, leading to a reconstruction of the Fermi surface topology. For intermediate doping levels, the realized stable electronic structure is a compromise between the solutions for the perfect lattice with y=0 and the vacancy stripe-ordered lattice with y=0.4, which results in a competition between vacancy random disorder and vacancy stripe order. A multiorbital hopping model is parameterized by comparing Fermi surface topologies to ARPES experiments, from which we construct a mean-field t-J lattice model to study the paramagnetic and antiferromagnetic (AFM) phases of K0.8Fe1.6Se2. In the AFM phase the calculated spin magnetization of the t-J model leads to a checker-board block-spin structure in good agreement with neutron scattering experiments and abinitio calculations.
Pressure-tuned quantum criticality in the antiferromagnetic Kondo semimetal CeNi2-δAs2.
Luo, Yongkang; Ronning, F; Wakeham, N; Lu, Xin; Park, Tuson; Xu, Z-A; Thompson, J D
2015-11-03
The easily tuned balance among competing interactions in Kondo-lattice metals allows access to a zero-temperature, continuous transition between magnetically ordered and disordered phases, a quantum-critical point (QCP). Indeed, these highly correlated electron materials are prototypes for discovering and exploring quantum-critical states. Theoretical models proposed to account for the strange thermodynamic and electrical transport properties that emerge around the QCP of a Kondo lattice assume the presence of an indefinitely large number of itinerant charge carriers. Here, we report a systematic transport and thermodynamic investigation of the Kondo-lattice system CeNi2-δAs2 (δ ≈ 0.28) as its antiferromagnetic order is tuned by pressure and magnetic field to zero-temperature boundaries. These experiments show that the very small but finite carrier density of ~0.032 E-/formular unit in CeNi2-δAs2 leads to unexpected transport signatures of quantum criticality and the delayed development of a fully coherent Kondo-lattice state with decreasing temperature. The small carrier density and associated semimetallicity of this Kondo-lattice material favor an unconventional, local-moment type of quantum criticality and raises the specter of the Nozières exhaustion idea that an insufficient number of conduction-electron spins to separately screen local moments requires collective Kondo screening.
Pressure-tuned quantum criticality in the antiferromagnetic Kondo semimetal CeNi2−δAs2
Luo, Yongkang; Ronning, F.; Wakeham, N.; Lu, Xin; Park, Tuson; Xu, Z.-A.; Thompson, J. D.
2015-01-01
The easily tuned balance among competing interactions in Kondo-lattice metals allows access to a zero-temperature, continuous transition between magnetically ordered and disordered phases, a quantum-critical point (QCP). Indeed, these highly correlated electron materials are prototypes for discovering and exploring quantum-critical states. Theoretical models proposed to account for the strange thermodynamic and electrical transport properties that emerge around the QCP of a Kondo lattice assume the presence of an indefinitely large number of itinerant charge carriers. Here, we report a systematic transport and thermodynamic investigation of the Kondo-lattice system CeNi2−δAs2 (δ ≈ 0.28) as its antiferromagnetic order is tuned by pressure and magnetic field to zero-temperature boundaries. These experiments show that the very small but finite carrier density of ∼0.032 e−/formular unit in CeNi2−δAs2 leads to unexpected transport signatures of quantum criticality and the delayed development of a fully coherent Kondo-lattice state with decreasing temperature. The small carrier density and associated semimetallicity of this Kondo-lattice material favor an unconventional, local-moment type of quantum criticality and raises the specter of the Nozières exhaustion idea that an insufficient number of conduction-electron spins to separately screen local moments requires collective Kondo screening. PMID:26483465
CVD diamond for electronic devices and sensors
2009-01-01
Synthetic diamond is diamond produced by using chemical or physical processes. Like naturally occurring diamond it is composed of a three-dimensional carbon crystal. Due to its extreme physical properties, synthetic diamond is used in many industrial applications, such as drill bits and scratch-proof coatings, and has the potential to be used in many new application areas A brand new title from the respected Wiley Materials for Electronic and Optoelectronic Applications series, this title is the most up-to-date resource for diamond specialists. Beginning with an introduction to the pr
Method for machining steel with diamond tools
Casstevens, John M.
1986-01-01
The present invention is directed to a method for machining optical quality inishes and contour accuracies of workpieces of carbon-containing metals such as steel with diamond tooling. The wear rate of the diamond tooling is significantly reduced by saturating the atmosphere at the interface of the workpiece and the diamond tool with a gaseous hydrocarbon during the machining operation. The presence of the gaseous hydrocarbon effectively eliminates the deterioration of the diamond tool by inhibiting or preventing the conversion of the diamond carbon to graphite carbon at the point of contact between the cutting tool and the workpiece.
Diamond Sensors for Energy Frontier Experiments
Schnetzer, Steve
2014-01-01
We discuss the use of diamond sensors in high-energy, high-i ntensity collider experiments. Re- sults from diamond sensor based beam conditions monitors in the ATLAS and CMS experiments at the CERN Large Hadron Collider (LHC) are presented and pla ns for diamond based luminosity monitors for the upcoming LHC run are described. We describe recent measurements on single crystal diamond sensors that indicate a polarization effec t that causes a reduction of charge col- lection efficiency as a function of particle flux. We conclude by describing new developments on the promising technology of 3D diamond sensors.
Nanocrystalline diamond films for biomedical applications
Pennisi, Cristian Pablo; Alcaide, Maria
2014-01-01
performance of nanocrystalline diamond films is reviewed from an application-specific perspective, covering topics such as enhancement of cellular adhesion, anti-fouling coatings, non-thrombogenic surfaces, micropatterning of cells and proteins, and immobilization of biomolecules for bioassays. In order......Nanocrystalline diamond films, which comprise the so called nanocrystalline diamond (NCD) and ultrananocrystalline diamond (UNCD), represent a class of biomaterials possessing outstanding mechanical, tribological, and electrical properties, which include high surface smoothness, high corrosion...... resistance, chemical inertness, superior electrochemical behavior, biocompatibility, and nontoxicity. These properties have positioned the nanocrystalline diamond films as an attractive class of materials for a range of therapeutic and diagnostic applications in the biomedical field. Consequently...
Transparent nanocrystalline diamond coatings and devices
Sumant, Anirudha V.; Khan, Adam
2017-08-22
A method for coating a substrate comprises producing a plasma ball using a microwave plasma source in the presence of a mixture of gases. The plasma ball has a diameter. The plasma ball is disposed at a first distance from the substrate and the substrate is maintained at a first temperature. The plasma ball is maintained at the first distance from the substrate, and a diamond coating is deposited on the substrate. The diamond coating has a thickness. Furthermore, the diamond coating has an optical transparency of greater than about 80%. The diamond coating can include nanocrystalline diamond. The microwave plasma source can have a frequency of about 915 MHz.
Electron Microscopy of Natural and Epitaxial Diamond
Posthill, J. B.; George, T.; Malta, D. P.; Humphreys, T. P.; Rudder, R. A.; Hudson, G. C.; Thomas, R. E.; Markunas, R. J.
1993-01-01
Semiconducting diamond films have the potential for use as a material in which to build active electronic devices capable of operating at high temperatures or in high radiation environments. Ultimately, it is preferable to use low-defect-density single crystal diamond for device fabrication. We have previously investigated polycrystalline diamond films with transmission electron microscopy (TEM) and scanning electron microscopy (SEM), and homoepitaxial films with SEM-based techniques. This contribution describes some of our most recent observations of the microstructure of natural diamond single crystals and homoepitaxial diamond thin films using TEM.
Selected Bibliography II-Diamond Surface Chemistry
1993-09-30
34Scanning Tunneling Microscopy of Polished Diamond Surfaces" JNL: Appl. Surf. Sci. REF: 62(4) (1992) 263-8 91 AUTHOR: Vazquez L., Martin -Gago J. A...Absorption in Semiconducting Synthetic Diamond" JNL: Physical Review REF: 140 (1965) A1272 AUTHOR: Keown R. TITLE: "Energy Bands in Diamond" JNL...34Determination of Optical Constant of Diamond Thin Films" JNL: Proc. SPIE-Int. Soc. Opt. Eng. REF: 1759(Diamond Opt. V) (1992) 218-23 AUTHOR: Fazzio A., Martins
Diamond Ablators for Inertial Confinement Fusion
Biener, J; Mirkarimi, P B; Tringe, J W; Baker, S L; Wang, Y M; Kucheyev, S O; Teslich, N E; Wu, K J; Hamza, A V; Wild, C; Woerner, E; Koidl, P; Bruehne, K; Fecht, H
2005-06-21
Diamond has a unique combination of physical properties for the inertial confinement fusion ablator application, such as appropriate optical properties, high atomic density, high yield strength, and high thermal conductivity. Here, we present a feasible concept to fabricate diamond ablator shells. The fabrication of diamond capsules is a multi-step process, which involves diamond chemical vapor deposition on silicon mandrels followed by polishing, microfabrication of holes, and removing of the silicon mandrel by an etch process. We also discuss the pros and cons of coarse-grained optical quality and nanocrystalline chemical vapor deposition diamond films for the ablator application.
Computational design of a robust two-dimensional antiferromagnetic semiconductor
Chabungbam, Satyananda; Sen, Prasenjit
2017-07-01
Using density functional theory calculations, we establish the hitherto unknown compound CrCTe3 to be a stable antiferromagnetic semiconductor in the R 3 ¯ crystal structure with an indirect fundamental gap. Successive layers in the bulk compound are weakly bound by van der Waals forces so that individual layers can be easily exfoliated. A monolayer of CrCTe3 is also an antiferromagnetic semiconductor. The monolayer is structurally stable over a large range of compressive and tensile strains, and the antiferromagnetic state is robust over this strain range. Band gap of the monolayer can be tuned by as much as 50% by applying strain in this range.
Magnonic analog of relativistic Zitterbewegung in an antiferromagnetic spin chain
Wang, Weiwei; Gu, Chenjie; Zhou, Yan; Fangohr, Hans
2017-07-01
We theoretically investigate the spin-wave (magnon) excitations in a classical antiferromagnetic spin chain with easy-axis anisotropy. We obtain a Dirac-like equation by linearizing the Landau-Lifshitz-Gilbert equation in this antiferromagnetic system, in contrast to the ferromagnetic system in which a Schrödinger-type equation is derived. The Hamiltonian operator in the Dirac-like equation is a pseudo-Hermitian. We compute and demonstrate relativistic Zitterbewegung (trembling motion) in the antiferromagnetic spin chain by measuring the expectation values of the wave-packet position.
Critical quasiparticles in single-impurity and lattice Kondo models
Vojta, M.; Bulla, R.; Wölfle, P.
2015-07-01
Quantum criticality in systems of local moments interacting with itinerant electrons has become an important and diverse field of research. Here we review recent results which concern (a) quantum phase transitions in single-impurity Kondo and Anderson models and (b) quantum phase transitions in heavy-fermion lattice models which involve critical quasiparticles. For (a) the focus will be on impurity models with a pseudogapped host density of states and their applications, e.g., in graphene and other Dirac materials, while (b) is devoted to strong-coupling behavior near antiferromagnetic quantum phase transitions, with potential applications in a variety of heavy-fermion metals.
Microplasma device architectures with various diamond nanostructures
Kunuku, Srinivasu; Jothiramalingam Sankaran, Kamatchi; Leou, Keh-Chyang; Lin, I.-Nan
2017-02-01
Diamond nanostructures (DNSs) were fabricated from three different morphological diamonds, microcrystalline diamond (MCD), nanocrystalline diamond (NCD), and ultrananocrystalline diamond (UNCD) films, using a reactive ion etching method. The plasma illumination (PI) behavior of microplasma devices using the DNSs and the diamond films as cathode were investigated. The Paschen curve approach revealed that the secondary electron emission coefficient (γ value) of diamond materials is similar irrespective of the microstructure (MCD, NCD, and UNCD) and geometry of the materials (DNSs and diamond films). The diamond materials show markedly larger γ-coefficient than conventional metallic cathode materials such as Mo that resulted in markedly better PI behavior for the corresponding microplasma devices. Moreover, the PI behavior, i.e. the voltage dependence of plasma current density (J pl‑V), plasma density (n e‑V), and the robustness of the devices, varied markedly with the microstructure and geometry of the cathode materials that was closely correlated to the electron field emission (EFE) properties of the cathode materials. The UNCD nanopillars, possessing good EFE properties, resulted in superior PI behavior, whereas the MCD diamond films with insufficient EFE properties led to inferior PI behavior. Consequently, enhancement of plasma characteristics is the collective effects of EFE behavior and secondary electron emission characteristics of diamond-based cathode materials.
Effects of diamond magnetism on the microstructure of electrodeposited diamond composites
Lu Huiyang; Li Yundong; Huang Zhiwei; Go Huiyan
2007-01-01
Electroformed diamond tools have been used for many years in grinding and cutting fields while electrodeposited diamond composite coatings have been widely studied due to their desirable hardness, wear and corrosion resistance. This article eports the detrimental impact of diamond magnetism on the composites microstructure and gives explanations. Microstructure differences between composites that, respectively, contained no - further - treated diamond, magnetism - strengthening treated diamond and magnetism weakening treated diamond were carefully observed. It is shown that diamond magnetization treatment drastically harms the composite microstructure (e. G. , roughening the coating surface, coarsening the matrix grain, and more seriously, reducing the mechanical retention of diamond grains in the matrix) while demagnetization treatment does the opposite. All the observed facts could be explained by the electromagnetic interaction between magnetic fields produced by magnetic diamond grains and electric current (moving cations) during the electrodeposition process.