Mechanical torques generated by optically pumped atomic spin relaxation at surfaces

Science.gov (United States)

Herman, R. M.

1982-03-01

It is argued that a valuable method of observing certain types of surface-atom interactions may lie in mechanical torques generated through the spin-orbit relaxation of valence electronic spins of optically pumped atoms at surfaces. The unusual feature of this phenomenon is that the less probable spin-orbit relaxation becomes highly visible as compared with the much more rapid paramagnetic relaxation, because of an enhancement, typically by as much as a factor 109, in the torques delivered to mechanical structures, by virtue of a very large effective moment arm. Spin-orbit relaxation operates through an exchange of translational momentum which, in turn, can be identified with the delivery of a gigantic angular momentum (in units of ℏ) relative to a distant axis about which mechanical motion is referred. The spin-orbit relaxation strongly depends upon the atomic number of the surface atoms and the strength of interaction with the optically pumped atoms. Being dominated by high-atomic-number surface atoms, spin-orbit-relaxation rates may not be too strongly influenced by minor surface contamination of lighter-weight optically active atoms.

Engineering the Eigenstates of Coupled Spin-1/2 Atoms on a Surface.

Science.gov (United States)

Yang, Kai; Bae, Yujeong; Paul, William; Natterer, Fabian D; Willke, Philip; Lado, Jose L; Ferrón, Alejandro; Choi, Taeyoung; Fernández-Rossier, Joaquín; Heinrich, Andreas J; Lutz, Christopher P

2017-12-01

Quantum spin networks having engineered geometries and interactions are eagerly pursued for quantum simulation and access to emergent quantum phenomena such as spin liquids. Spin-1/2 centers are particularly desirable, because they readily manifest coherent quantum fluctuations. Here we introduce a controllable spin-1/2 architecture consisting of titanium atoms on a magnesium oxide surface. We tailor the spin interactions by atomic-precision positioning using a scanning tunneling microscope (STM) and subsequently perform electron spin resonance on individual atoms to drive transitions into and out of quantum eigenstates of the coupled-spin system. Interactions between the atoms are mapped over a range of distances extending from highly anisotropic dipole coupling to strong exchange coupling. The local magnetic field of the magnetic STM tip serves to precisely tune the superposition states of a pair of spins. The precise control of the spin-spin interactions and ability to probe the states of the coupled-spin network by addressing individual spins will enable the exploration of quantum many-body systems based on networks of spin-1/2 atoms on surfaces.

Spin valve effect in single-atom contacts

International Nuclear Information System (INIS)

Ziegler, M; Neel, N; Berndt, R; Lazo, C; Ferriani, P; Heinze, S; Kroeger, J

2011-01-01

Magnetic single-atom contacts have been controllably fabricated with a scanning tunnelling microscope. A voltage-dependent spin valve effect with conductance variations of ∼40% is reproducibly observed from contacts comprising a Cr-covered tip and Co and Cr atoms on ferromagnetic nanoscale islands on W(110) with opposite magnetization. The spin-dependent conductances are interpreted from first-principles calculations in terms of the orbital character of the relevant electronic states of the junction.

Spin squeezing and Schrödinger cat generation in atomic samples with Rydberg blockade

DEFF Research Database (Denmark)

Opatrný, Tomáš; Mølmer, Klaus

2012-01-01

A scheme is proposed to prepare squeezed states and Schrödinger-cat-like states of the collective spin degrees of freedom associated with a pair of ground states in an atomic ensemble. The scheme uses an effective Jaynes-Cummings interaction which can be provided by excitation of the atoms...

Majorana spin in magnetic atomic chain systems

Science.gov (United States)

Li, Jian; Jeon, Sangjun; Xie, Yonglong; Yazdani, Ali; Bernevig, B. Andrei

2018-03-01

In this paper, we establish that Majorana zero modes emerging from a topological band structure of a chain of magnetic atoms embedded in a superconductor can be distinguished from trivial localized zero energy states that may accidentally form in this system using spin-resolved measurements. To demonstrate this key Majorana diagnostics, we study the spin composition of magnetic impurity induced in-gap Shiba states in a superconductor using a hybrid model. By examining the spin and spectral densities in the context of the Bogoliubov-de Gennes (BdG) particle-hole symmetry, we derive a sum rule that relates the spin densities of localized Shiba states with those in the normal state without superconductivity. Extending our investigations to a ferromagnetic chain of magnetic impurities, we identify key features of the spin properties of the extended Shiba state bands, as well as those associated with a localized Majorana end mode when the effect of spin-orbit interaction is included. We then formulate a phenomenological theory for the measurement of the local spin densities with spin-polarized scanning tunneling microscopy (STM) techniques. By combining the calculated spin densities and the measurement theory, we show that spin-polarized STM measurements can reveal a sharp contrast in spin polarization between an accidental-zero-energy trivial Shiba state and a Majorana zero mode in a topological superconducting phase in atomic chains. We further confirm our results with numerical simulations that address generic parameter settings.

Probing quantum coherence in single-atom electron spin resonance

Science.gov (United States)

Willke, Philip; Paul, William; Natterer, Fabian D.; Yang, Kai; Bae, Yujeong; Choi, Taeyoung; Fernández-Rossier, Joaquin; Heinrich, Andreas J.; Lutz, Christoper P.

2018-01-01

Spin resonance of individual spin centers allows applications ranging from quantum information technology to atomic-scale magnetometry. To protect the quantum properties of a spin, control over its local environment, including energy relaxation and decoherence processes, is crucial. However, in most existing architectures, the environment remains fixed by the crystal structure and electrical contacts. Recently, spin-polarized scanning tunneling microscopy (STM), in combination with electron spin resonance (ESR), allowed the study of single adatoms and inter-atomic coupling with an unprecedented combination of spatial and energy resolution. We elucidate and control the interplay of an Fe single spin with its atomic-scale environment by precisely tuning the phase coherence time T2 using the STM tip as a variable electrode. We find that the decoherence rate is the sum of two main contributions. The first scales linearly with tunnel current and shows that, on average, every tunneling electron causes one dephasing event. The second, effective even without current, arises from thermally activated spin-flip processes of tip spins. Understanding these interactions allows us to maximize T2 and improve the energy resolution. It also allows us to maximize the amplitude of the ESR signal, which supports measurements even at elevated temperatures as high as 4 K. Thus, ESR-STM allows control of quantum coherence in individual, electrically accessible spins. PMID:29464211

Inertial rotation measurement with atomic spins: From angular momentum conservation to quantum phase theory

Science.gov (United States)

Zhang, C.; Yuan, H.; Tang, Z.; Quan, W.; Fang, J. C.

2016-12-01

Rotation measurement in an inertial frame is an important technology for modern advanced navigation systems and fundamental physics research. Inertial rotation measurement with atomic spin has demonstrated potential in both high-precision applications and small-volume low-cost devices. After rapid development in the last few decades, atomic spin gyroscopes are considered a promising competitor to current conventional gyroscopes—from rate-grade to strategic-grade applications. Although it has been more than a century since the discovery of the relationship between atomic spin and mechanical rotation by Einstein [Naturwissenschaften, 3(19) (1915)], research on the coupling between spin and rotation is still a focus point. The semi-classical Larmor precession model is usually adopted to describe atomic spin gyroscope measurement principles. More recently, the geometric phase theory has provided a different view of the rotation measurement mechanism via atomic spin. The theory has been used to describe a gyroscope based on the nuclear spin ensembles in diamond. A comprehensive understanding of inertial rotation measurement principles based on atomic spin would be helpful for future applications. This work reviews different atomic spin gyroscopes and their rotation measurement principles with a historical overlook. In addition, the spin-rotation coupling mechanism in the context of the quantum phase theory is presented. The geometric phase is assumed to be the origin of the measurable rotation signal from atomic spins. In conclusion, with a complete understanding of inertial rotation measurements using atomic spin and advances in techniques, wide application of high-performance atomic spin gyroscopes is expected in the near future.

Hydrodynamics of Normal Atomic Gases with Spin-orbit Coupling.

Science.gov (United States)

Hou, Yan-Hua; Yu, Zhenhua

2015-10-20

Successful realization of spin-orbit coupling in atomic gases by the NIST scheme opens the prospect of studying the effects of spin-orbit coupling on many-body physics in an unprecedentedly controllable way. Here we derive the linearized hydrodynamic equations for the normal atomic gases of the spin-orbit coupling by the NIST scheme with zero detuning. We show that the hydrodynamics of the system crucially depends on the momentum susceptibilities which can be modified by the spin-orbit coupling. We reveal the effects of the spin-orbit coupling on the sound velocities and the dipole mode frequency of the gases by applying our formalism to the ideal Fermi gas. We also discuss the generalization of our results to other situations.

Laser driven source of spin polarized atomic deuterium and hydrogen

International Nuclear Information System (INIS)

Poelker, M.; Coulter, K.P.; Holt, R.J.

1993-01-01

Optical pumping of potassium atoms in the presence of a high magnetic field followed by spin exchange collisions with deuterium (hydrogen) is shown to yield a high flux of spin polarized atomic deuterium (hydrogen). The performance of the laser driven source has been characterized as a function of deuterium (hydrogen) flow rate, potassium density, pump laser power, and magnetic field. Under appropriate conditions, the authors have observed deuterium atomic polarization as high as 75% at a flow rate 4.2x10 17 atoms/second. Preliminary results suggest that high nuclear polarizations are obtained in the absence of weak field rf transitions as a result of a spin temperature distribution that evolves through frequent H-H (D-D) collisions

Sensitivity optimization of Bell-Bloom magnetometers by manipulation of atomic spin synchronization

Science.gov (United States)

Ranjbaran, M.; Tehranchi, M. M.; Hamidi, S. M.; Khalkhali, S. M. H.

2018-05-01

Many efforts have been devoted to the developments of atomic magnetometers for achieving the high sensitivity required in biomagnetic applications. To reach the high sensitivity, many types of atomic magnetometers have been introduced for optimization of the creation and relaxation rates of atomic spin polarization. In this paper, regards to sensitivity optimization techniques in the Mx configuration, we have proposed a novelty approach for synchronization of the spin precession in the Bell-Bloom magnetometers. We have utilized the phenomenological Bloch equations to simulate the spin dynamics when modulation of pumping light and radio frequency magnetic field were both used for atomic spin synchronization. Our results showed that the synchronization process, improved the magnetometer sensitivity respect to the classical configurations.

Recent advances in atomic-scale spin-polarized scanning tunneling microscopy.

Science.gov (United States)

Smith, Arthur R; Yang, Rong; Yang, Haiqiang; Dick, Alexey; Neugebauer, Joerg; Lambrecht, Walter R L

2005-02-01

The Mn3N2 (010) surface has been studied using spin-polarized scanning tunneling microscopy at the atomic scale. The principle objective of this work is to elucidate the properties and potential of this technique to measure atomic-scale magnetic structures. The experimental approach involves the use of a combined molecular beam epitaxy/scanning tunneling microscopy system that allows the study of atomically clean magnetic surfaces. Several key findings have been obtained. First, both magnetic and non-magnetic atomic-scale information has been obtained in a single spin-polarized image. Magnetic modulation of the height profile having an antiferromagnetic super-period of c = 12.14 A (6 atomic rows) together with a non-magnetic superstructure having a period of c/2 = 6.07 A (3 atomic rows) was observed. Methods of separation of magnetic and non-magnetic profiles are presented. Second, bias voltage-dependent spin-polarized images show a reversal of the magnetic modulation at a particular voltage. This reversal is clearly due to a change in the sign of the magnetic term in the tunnel current. Since this term depends on both the tip's as well as the sample's magnetic local density of states, the reversal can be caused by either the sample or the tip. Third, the shape of the line profile was found to vary with the bias voltage, which is related to the energy-dependent spin contribution from the 2 chemically inequivalent Mn sites on the surface. Overall, the results shown here expand the application of the method of spin-polarized scanning tunneling microscopy to measure atomic-scale magnetic structures. (c) 2005 Wiley-Liss, Inc.

Negative-Mass Instability of the Spin and Motion of an Atomic Gas Driven by Optical Cavity Backaction

Science.gov (United States)

Kohler, Jonathan; Gerber, Justin A.; Dowd, Emma; Stamper-Kurn, Dan M.

2018-01-01

We realize a spin-orbit interaction between the collective spin precession and center-of-mass motion of a trapped ultracold atomic gas, mediated by spin- and position-dependent dispersive coupling to a driven optical cavity. The collective spin, precessing near its highest-energy state in an applied magnetic field, can be approximated as a negative-mass harmonic oscillator. When the Larmor precession and mechanical motion are nearly resonant, cavity mediated coupling leads to a negative-mass instability, driving exponential growth of a correlated mode of the hybrid system. We observe this growth imprinted on modulations of the cavity field and estimate the full covariance of the resulting two-mode state by observing its transient decay during subsequent free evolution.

Concept for room temperature single-spin tunneling force microscopy with atomic spatial resolution

Science.gov (United States)

Payne, Adam

A study of a force detected single-spin magnetic resonance measurement concept with atomic spatial resolution is presented. The method is based upon electrostatic force detection of spin-selection rule controlled single electron tunneling between two electrically isolated paramagnetic states. Single-spin magnetic resonance detection is possible by measuring the force detected tunneling charge noise on and off spin resonance. Simulation results of this charge noise, based upon physical models of the tunneling and spin physics, are directly compared to measured atomic force microscopy (AFM) system noise. The results show that the approach could provide single-spin measurement of electrically isolated defect states with atomic spatial resolution at room temperature.

Atomic-resolution single-spin magnetic resonance detection concept based on tunneling force microscopy

Science.gov (United States)

Payne, A.; Ambal, K.; Boehme, C.; Williams, C. C.

2015-05-01

A study of a force detected single-spin magnetic resonance measurement concept with atomic spatial resolution is presented. The method is based upon electrostatic force detection of spin-selection rule controlled single-electron tunneling between two electrically isolated paramagnetic states. Single-spin magnetic resonance detection is possible by measuring the force detected tunneling charge noise on and off spin resonance. Simulation results of this charge noise, based upon physical models of the tunneling and spin physics, are directly compared to measured atomic force microscopy system noise. The results show that the approach could provide single-spin measurement of electrically isolated qubit states with atomic spatial resolution at room temperature.

Fermionic Collective Excitations in a Lattice Gas of Rydberg Atoms

International Nuclear Information System (INIS)

Olmos, B.; Gonzalez-Ferez, R.; Lesanovsky, I.

2009-01-01

We investigate the many-body quantum states of a laser-driven gas of Rydberg atoms confined to a large spacing ring lattice. If the laser driving is much stronger than the van der Waals interaction among the Rydberg atoms, these many-body states are collective fermionic excitations. The first excited state is a spin wave that extends over the entire lattice. We demonstrate that our system permits us to study fermions in the presence of disorder although no external atomic motion takes place. We analyze how this disorder influences the excitation properties of the fermionic states. Our work shows a route towards the creation of complex many-particle states with atoms in lattices.

Long-lived qubit from three spin-(1/2) atoms

International Nuclear Information System (INIS)

Han Rui; Loerch, Niels; Suzuki, Jun; Englert, Berthold-Georg

2011-01-01

A system of three spin-(1/2) atoms allows the construction of a reference-frame-free (RFF) qubit in the subspace with total angular momentum j=1/2. The RFF qubit stays coherent perfectly as long as the spins of the three atoms are affected homogeneously. The inhomogeneous evolution of the atoms causes decoherence, but this decoherence can be suppressed efficiently by applying a bias magnetic field of modest strength perpendicular to the plane of the atoms. The resulting lifetime of the RFF qubit can be many days, making RFF qubits of this kind promising candidates for quantum information storage units. Specifically, we examine the situation of three 6 Li atoms trapped in a CO 2 -laser-generated optical lattice and find that, with conservatively estimated parameters, a stored qubit maintains a fidelity of 0.9999 for two hours.

Polarization transfer from polarized nuclear spin to μ- spin in muonic atom

International Nuclear Information System (INIS)

Kuno, Yoshitaka; Nagamine, Kanetada; Yamazaki, Toshimitsu.

1987-02-01

A theoretical study of polarization transfer from an initially-polarized nuclear spin to a μ - spin in a muonic atom is given. The switching of the hyperfine interaction at excited muonic states as well as at the ground 1s state is taken into account. The upper state of hyperfine doublet at the muonic 1s state is considered to proceed down to the lower state. It is found that as the hyperfine interaction becomes effective at higher excited muonic orbitals, a less extent of polarization is transferred from the nuclear spin to the μ - spin. The theoretical values obtained are compared with the recent experiment of μ - repolarization in a polarized 209 Bi target. (author)

The magnetism and spin-dependent electronic transport properties of boron nitride atomic chains

International Nuclear Information System (INIS)

An, Yipeng; Zhang, Mengjun; Wang, Tianxing; Jiao, Zhaoyong; Wu, Dapeng; Fu, Zhaoming; Wang, Kun

2016-01-01

Very recently, boron nitride atomic chains were successively prepared and observed in experiments [O. Cretu et al., ACS Nano 8, 11950 (2015)]. Herein, using a first-principles technique, we study the magnetism and spin-dependent electronic transport properties of three types of BN atomic chains whose magnetic moment is 1 μ B for B n N n−1 , 2 μ B for B n N n , and 3 μ B for B n N n+1 type atomic chains, respectively. The spin-dependent electronic transport results demonstrate that the short B n N n+1 chain presents an obvious spin-filtering effect with high spin polarization ratio (>90%) under low bias voltages. Yet, this spin-filtering effect does not occur for long B n N n+1 chains under high bias voltages and other types of BN atomic chains (B n N n−1 and B n N n ). The proposed short B n N n+1 chain is predicted to be an effective low-bias spin filters. Moreover, the length-conductance relationships of these BN atomic chains were also studied.

Observation of multicellular spinning behavior of Proteus mirabilis by atomic force microscopy and multifunctional microscopy.

Science.gov (United States)

Liu, Yanxia; Deng, Yuanxin; Luo, Shuxiu; Deng, Yu; Guo, Linming; Xu, Weiwei; Liu, Lei; Liu, Junkang

2014-01-01

This study aimed to observe the multicellular spinning behavior of Proteus mirabilis by atomic force microscopy (AFM) and multifunctional microscopy in order to understand the mechanism underlying this spinning movement and its biological significance. Multifunctional microscopy with charge-coupled device (CCD) and real-time AFM showed changes in cell structure and shape of P. mirabilis during multicellular spinning movement. Specifically, the morphological characteristics of P. mirabilis, multicellular spinning dynamics, and unique movement were observed. Our findings indicate that the multicellular spinning behavior of P. mirabilis may be used to collect nutrients, perform colonization, and squeeze out competitors. The movement characteristics of P. mirabilis are vital to the organism's biological adaptability to the surrounding environment. Copyright © 2013 Elsevier Ltd. All rights reserved.

Entangling two transportable neutral atoms via local spin exchange.

Science.gov (United States)

Kaufman, A M; Lester, B J; Foss-Feig, M; Wall, M L; Rey, A M; Regal, C A

2015-11-12

To advance quantum information science, physical systems are sought that meet the stringent requirements for creating and preserving quantum entanglement. In atomic physics, robust two-qubit entanglement is typically achieved by strong, long-range interactions in the form of either Coulomb interactions between ions or dipolar interactions between Rydberg atoms. Although such interactions allow fast quantum gates, the interacting atoms must overcome the associated coupling to the environment and cross-talk among qubits. Local interactions, such as those requiring substantial wavefunction overlap, can alleviate these detrimental effects; however, such interactions present a new challenge: to distribute entanglement, qubits must be transported, merged for interaction, and then isolated for storage and subsequent operations. Here we show how, using a mobile optical tweezer, it is possible to prepare and locally entangle two ultracold neutral atoms, and then separate them while preserving their entanglement. Ground-state neutral atom experiments have measured dynamics consistent with spin entanglement, and have detected entanglement with macroscopic observables; we are now able to demonstrate position-resolved two-particle coherence via application of a local gradient and parity measurements. This new entanglement-verification protocol could be applied to arbitrary spin-entangled states of spatially separated atoms. The local entangling operation is achieved via spin-exchange interactions, and quantum tunnelling is used to combine and separate atoms. These techniques provide a framework for dynamically entangling remote qubits via local operations within a large-scale quantum register.

Dynamical Negative Differential Resistance in Antiferromagnetically Coupled Few-Atom Spin Chains

Science.gov (United States)

Rolf-Pissarczyk, Steffen; Yan, Shichao; Malavolti, Luigi; Burgess, Jacob A. J.; McMurtrie, Gregory; Loth, Sebastian

2017-11-01

We present the appearance of negative differential resistance (NDR) in spin-dependent electron transport through a few-atom spin chain. A chain of three antiferromagnetically coupled Fe atoms (Fe trimer) was positioned on a Cu2 N /Cu (100 ) surface and contacted with the spin-polarized tip of a scanning tunneling microscope, thus coupling the Fe trimer to one nonmagnetic and one magnetic lead. Pronounced NDR appears at the low bias of 7 mV, where inelastic electron tunneling dynamically locks the atomic spin in a long-lived excited state. This causes a rapid increase of the magnetoresistance between the spin-polarized tip and Fe trimer and quenches elastic tunneling. By varying the coupling strength between the tip and Fe trimer, we find that in this transport regime the dynamic locking of the Fe trimer competes with magnetic exchange interaction, which statically forces the Fe trimer into its high-magnetoresistance state and removes the NDR.

Atomic-Scale Nuclear Spin Imaging Using Quantum-Assisted Sensors in Diamond

Directory of Open Access Journals (Sweden)

A. Ajoy

2015-01-01

Full Text Available Nuclear spin imaging at the atomic level is essential for the understanding of fundamental biological phenomena and for applications such as drug discovery. The advent of novel nanoscale sensors promises to achieve the long-standing goal of single-protein, high spatial-resolution structure determination under ambient conditions. In particular, quantum sensors based on the spin-dependent photoluminescence of nitrogen-vacancy (NV centers in diamond have recently been used to detect nanoscale ensembles of external nuclear spins. While NV sensitivity is approaching single-spin levels, extracting relevant information from a very complex structure is a further challenge since it requires not only the ability to sense the magnetic field of an isolated nuclear spin but also to achieve atomic-scale spatial resolution. Here, we propose a method that, by exploiting the coupling of the NV center to an intrinsic quantum memory associated with the nitrogen nuclear spin, can reach a tenfold improvement in spatial resolution, down to atomic scales. The spatial resolution enhancement is achieved through coherent control of the sensor spin, which creates a dynamic frequency filter selecting only a few nuclear spins at a time. We propose and analyze a protocol that would allow not only sensing individual spins in a complex biomolecule, but also unraveling couplings among them, thus elucidating local characteristics of the molecule structure.

New directions in the theory of spin-polarized atomic hydrogen and deuterium

International Nuclear Information System (INIS)

Koelman, J.M.V.A.

1988-01-01

The three chapters of this thesis dealing with collisions between hydrogen (or deuterium) atoms in their ground state, each treat a different development in the theory of atomic hydrogen or deuterium gas. The decay due to interatomic collisions hindered till now all attempts to reach the low temperature, high-density regime where effects due to degeneracy are expected to show up. In ch. 2 a simple way out is presented for the case of Fermi gases: In spin-polarized Fermi systems at very low temperatures collisions are much effective than in Bose systems. For the Fermi gas, consisting of magnetically confined deuterium atoms, it appears that fast spin-exchange collisions automatically lead to a completely spin-polarized gas for which the spin-relaxation limited lifetime increases dramatically with decreasing temperature. As also the ratio of internal thermalization rate over decay rate increases with decreasing temperature, this gas can be cooled by forced evaporation down to very low temperatures. In ch. 3 it iis shown that the nuclear spin dynamics due to the hyperfine interaction during collisions, strongly limits the improvement in frequency stability attainable by H masers operating at low temperatures. In ch. 4 the phenomenon of spin waves is studied. It is shown that, despite the fact that interactions between two atoms are nuclear-spin independent, the outcome of a scattering event does not depend on the nuclear spins involved due to the particle indistinguishability effects at low collision energies. This effect gives rise to quantum phenomena on a macroscopic scale via the occurrence of spin waves. (author). 185 refs.; 34 figs

Spin-splitting calculation for zincblende semiconductors using an atomic bond-orbital model

International Nuclear Information System (INIS)

Kao, Hsiu-Fen; Lo, Ikai; Chiang, Jih-Chen; Wang, Wan-Tsang; Hsu, Yu-Chi; Wu, Chieh-Lung; Gau, Ming-Hong; Chen, Chun-Nan; Ren, Chung-Yuan; Lee, Meng-En

2012-01-01

We develop a 16-band atomic bond-orbital model (16ABOM) to compute the spin splitting induced by bulk inversion asymmetry in zincblende materials. This model is derived from the linear combination of atomic-orbital (LCAO) scheme such that the characteristics of the real atomic orbitals can be preserved to calculate the spin splitting. The Hamiltonian of 16ABOM is based on a similarity transformation performed on the nearest-neighbor LCAO Hamiltonian with a second-order Taylor expansion over k-vector at the Γ point. The spin-splitting energies in bulk zincblende semiconductors, GaAs and InSb, are calculated, and the results agree with the LCAO and first-principles calculations. However, we find that the spin-orbit coupling between bonding and antibonding p-like states, evaluated by the 16ABOM, dominates the spin splitting of the lowest conduction bands in the zincblende materials.

A numerical study of spin-dependent organization of alkali-metal atomic clusters using density-functional method

International Nuclear Information System (INIS)

Liu Xuan; Ito, Haruhiko; Torikai, Eiko

2012-01-01

We calculate the different geometric isomers of spin clusters composed of a small number of alkali-metal atoms using the UB3LYP density-functional method. The electron density distribution of clusters changes according to the value of total spin. Steric structures as well as planar structures arise when the number of atoms increases. The lowest spin state is the most stable and Li n , Na n , K n , Rb n , and Cs n with n = 2–8 can be formed in higher spin states. In the highest spin state, the preparation of clusters depends on the kind and the number of constituent atoms. The interaction energy between alkali-metal atoms and rare-gas atoms is smaller than the binding energy of spin clusters. Consequently, it is possible to self-organize the alkali-metal-atom clusters on a non-wetting substrate coated with rare-gas atoms.

A numerical study of spin-dependent organization of alkali-metal atomic clusters using density-functional method

Energy Technology Data Exchange (ETDEWEB)

Liu Xuan, E-mail: liu.x.ad@m.titech.ac.jp; Ito, Haruhiko [Interdisciplinary Graduate School of Science and Engineering, Tokyo Institute of Technology (Japan); Torikai, Eiko [Interdisciplinary Graduate School of Medicine and Engineering, University of Yamanashi (Japan)

2012-08-15

We calculate the different geometric isomers of spin clusters composed of a small number of alkali-metal atoms using the UB3LYP density-functional method. The electron density distribution of clusters changes according to the value of total spin. Steric structures as well as planar structures arise when the number of atoms increases. The lowest spin state is the most stable and Li{sub n}, Na{sub n}, K{sub n}, Rb{sub n}, and Cs{sub n} with n = 2-8 can be formed in higher spin states. In the highest spin state, the preparation of clusters depends on the kind and the number of constituent atoms. The interaction energy between alkali-metal atoms and rare-gas atoms is smaller than the binding energy of spin clusters. Consequently, it is possible to self-organize the alkali-metal-atom clusters on a non-wetting substrate coated with rare-gas atoms.

Single-passage read-out of atomic quantum memory

DEFF Research Database (Denmark)

Fiurasek, J; Sherson, J; Opatrny, T

2005-01-01

Retrieving quantum information, collective atomic spin systems, quantum memory Udgivelsesdato: 17 Feb.......Retrieving quantum information, collective atomic spin systems, quantum memory Udgivelsesdato: 17 Feb....

Nonlocally sensing the magnetic states of nanoscale antiferromagnets with an atomic spin sensor.

Science.gov (United States)

Yan, Shichao; Malavolti, Luigi; Burgess, Jacob A J; Droghetti, Andrea; Rubio, Angel; Loth, Sebastian

2017-05-01

The ability to sense the magnetic state of individual magnetic nano-objects is a key capability for powerful applications ranging from readout of ultradense magnetic memory to the measurement of spins in complex structures with nanometer precision. Magnetic nano-objects require extremely sensitive sensors and detection methods. We create an atomic spin sensor consisting of three Fe atoms and show that it can detect nanoscale antiferromagnets through minute, surface-mediated magnetic interaction. Coupling, even to an object with no net spin and having vanishing dipolar stray field, modifies the transition matrix element between two spin states of the Fe atom-based spin sensor that changes the sensor's spin relaxation time. The sensor can detect nanoscale antiferromagnets at up to a 3-nm distance and achieves an energy resolution of 10 μeV, surpassing the thermal limit of conventional scanning probe spectroscopy. This scheme permits simultaneous sensing of multiple antiferromagnets with a single-spin sensor integrated onto the surface.

Thin film coatings which inhibit spin relaxation of polarized potassium atoms

International Nuclear Information System (INIS)

Thomas, G.E.; Holt, R.J.; Boyer, D.; Green, M.C.; Kowalczyk, R.S.; Young, L.

1986-01-01

A prototype of a polarized deuterium target which employs the spin exchange method is being developed. The mixing cell for mixing deuterium atoms and potassium vapor requires a surface that will reflect these atoms without being destroyed by the corrosive potassium. Thin film coating methods and a technique for coating pyrex are described. Results of spin relaxation measurements are given

Quantum Phase Transition in a Cold Atomic Spin-Boson Mixture

Science.gov (United States)

Orth, Peter P.; Stanic, Ivan; Le Hur, Karyn

2008-03-01

We theoretically implement a spin array in a tunable bosonic environment using cold bosonic atoms with two (hyperfine) ground states, trapped by different potentials [1]. The first specie lies in a deep optical lattice with tightly confining wells and forms a spin array; spin-up/down corresponds to occupation by one/no atom at each site. The second specie forms a superfluid reservoir. Different species are coupled coherently via laser transitions and collisions. Whereas the laser coupling mimics a transverse field for the spins, the coupling to the reservoir phonons (sound modes) induces a ferromagnetic (Ising) coupling as well as dissipation. This results in a peculiar ferro-paramagnetic quantum phase transition where the effect of dissipation can be studied in a controllable manner. [1] Peter P. Orth, Ivan Stanic, and Karyn Le Hur, arXiv:0711.2309 [cond-mat.other].

Long Spin-Relaxation Times in a Transition-Metal Atom in Direct Contact to a Metal Substrate.

Science.gov (United States)

Hermenau, Jan; Ternes, Markus; Steinbrecher, Manuel; Wiesendanger, Roland; Wiebe, Jens

2018-03-14

Long spin-relaxation times are a prerequisite for the use of spins in data storage or nanospintronics technologies. An atomic-scale solid-state realization of such a system is the spin of a transition-metal atom adsorbed on a suitable substrate. For the case of a metallic substrate, which enables the direct addressing of the spin by conduction electrons, the experimentally measured lifetimes reported to date are on the order of only hundreds of femtoseconds. Here, we show that the spin states of iron atoms adsorbed directly on a conductive platinum substrate have a surprisingly long spin-relaxation time in the nanosecond regime, which is comparable to that of a transition metal atom decoupled from the substrate electrons by a thin decoupling layer. The combination of long spin-relaxation times and strong coupling to conduction electrons implies the possibility to use flexible coupling schemes to process the spin information.

Magnetic Interaction between Surface-Engineered Rare-Earth Atomic Spins

Directory of Open Access Journals (Sweden)

Chiung-Yuan Lin

2012-06-01

Full Text Available We report the ab-initio study of rare-earth adatoms (Gd on an insulating surface. This surface is of interest because of previous studies by scanning tunneling microscopy showing spin excitations of transition-metal adatoms. The present work is the first study of rare-earth spin-coupled adatoms, as well as the geometry effect of spin coupling and the underlying mechanism of ferromagnetic coupling. The exchange coupling between Gd atoms on the surface is calculated to be antiferromagnetic in a linear geometry and ferromagnetic in a diagonal geometry. We also find that the Gd dimers in these two geometries are similar to the nearest-neighbor and the next-nearest-neighbor Gd atoms in GdN bulk. We analyze how much direct exchange, superexchange, and Ruderman-Kittel-Kasuya-Yosida interactions contribute to the exchange coupling for both geometries by additional first-principles calculations of related model systems.

Engineering the Dynamics of Effective Spin-Chain Models for Strongly Interacting Atomic Gases

DEFF Research Database (Denmark)

Volosniev, A. G.; Petrosyan, D.; Valiente, M.

2015-01-01

We consider a one-dimensional gas of cold atoms with strong contact interactions and construct an effective spin-chain Hamiltonian for a two-component system. The resulting Heisenberg spin model can be engineered by manipulating the shape of the external confining potential of the atomic gas. We...

Spin Squeezing and Entanglement with Room Temperature Atoms for Quantum Sensing and Communication

DEFF Research Database (Denmark)

Shen, Heng

magnetometer at room temperature is reported. Furthermore, using spin-squeezing of atomic ensemble, the sensitivity of magnetometer is improved. Deterministic continuous variable teleportation between two distant atomic ensembles is demonstrated. The fidelity of teleportating dynamically changing sequence...... of spin states surpasses a classical benchmark, demonstrating the true quantum teleportation....

Antihydrogen atom formation in a CUSP trap towards spin polarized beams

Energy Technology Data Exchange (ETDEWEB)

Kuroda, N., E-mail: kuroda@radphys4.c.u-tokyo.ac.jp [University of Tokyo, Graduate School of Arts and Sciences (Japan); Enomoto, Y. [RIKEN Advanced Science Institute (Japan); Michishio, K. [Tokyo University of Science, Department of Physics (Japan); Kim, C. H. [University of Tokyo, Graduate School of Arts and Sciences (Japan); Higaki, H. [Hiroshima University, Graduate School of Advanced Science of Matter (Japan); Nagata, Y.; Kanai, Y. [RIKEN Advanced Science Institute (Japan); Torii, H. A. [University of Tokyo, Graduate School of Arts and Sciences (Japan); Corradini, M.; Leali, M.; Lodi-Rizzini, E.; Venturelli, L.; Zurlo, N. [Universita di Brescia and Instituto Nazionale di Fisica Nucleare, Dipartimento di Chimica e Fisica per l' Ingegneria e per i Materiali (Italy); Fujii, K.; Ohtsuka, M.; Tanaka, K. [University of Tokyo, Graduate School of Arts and Sciences (Japan); Imao, H. [RIKEN Nishina Center for Accelerator-Based Science (Japan); Nagashima, Y. [Tokyo University of Science, Department of Physics (Japan); Matsuda, Y. [University of Tokyo, Graduate School of Arts and Sciences (Japan); Juhasz, B. [Stefan Meyer Institut fuer Subatomare Physik (Austria); and others

2012-12-15

The ASACUSA collaboration has been making a path to realize high precision microwave spectroscopy of ground-state hyperfine transitions of antihydrogen atom in flight for stringent test of the CPT symmetry. For this purpose, an efficient extraction of a spin polarized antihydrogen beam is essential. In 2010, we have succeeded in synthesizing our first cold antihydrogen atoms employing a CUSP trap. The CUSP trap confines antiprotons and positrons simultaneously with its axially symmetric magnetic field to form antihydrogen atoms. It is expected that antihydrogen atoms in the low-field-seeking states are preferentially focused along the cusp magnetic field axis whereas those in the high-field-seeking states are defocused, resulting in the formation of a spin-polarized antihydrogen beam.

Spin-dependent electronic transport properties of transition metal atoms doped α-armchair graphyne nanoribbons

Science.gov (United States)

Fotoohi, Somayeh; Haji-Nasiri, Saeed

2018-04-01

Spin-dependent electronic transport properties of single 3d transition metal (TM) atoms doped α-armchair graphyne nanoribbons (α-AGyNR) are investigated by non-equilibrium Green's function (NEGF) method combined with density functional theory (DFT). It is found that all of the impurity atoms considered in this study (Fe, Co, Ni) prefer to occupy the sp-hybridized C atom site in α-AGyNR, and the obtained structures remain planar. The results show that highly localized impurity states are appeared around the Fermi level which correspond to the 3d orbitals of TM atoms, as can be derived from the projected density of states (PDOS). Moreover, Fe, Co, and Ni doped α-AGyNRs exhibit magnetic properties due to the strong spin splitting property of the energy levels. Also for each case, the calculated current-voltage characteristic per super-cell shows that the spin degeneracy in the system is obviously broken and the current becomes strongly spin dependent. Furthermore, a high spin-filtering effect around 90% is found under the certain bias voltages in Ni doped α-AGyNR. Additionally, the structure with Ni impurity reveals transfer characteristic that is suitable for designing a spin current switch. Our findings provide a high possibility to design the next generation spin nanodevices with novel functionalities.

Modeling and optimizing of the random atomic spin gyroscope drift based on the atomic spin gyroscope

Energy Technology Data Exchange (ETDEWEB)

Quan, Wei; Lv, Lin, E-mail: lvlinlch1990@163.com; Liu, Baiqi [School of Instrument Science and Opto-Electronics Engineering, Beihang University, Beijing 100191 (China)

2014-11-15

In order to improve the atom spin gyroscope's operational accuracy and compensate the random error caused by the nonlinear and weak-stability characteristic of the random atomic spin gyroscope (ASG) drift, the hybrid random drift error model based on autoregressive (AR) and genetic programming (GP) + genetic algorithm (GA) technique is established. The time series of random ASG drift is taken as the study object. The time series of random ASG drift is acquired by analyzing and preprocessing the measured data of ASG. The linear section model is established based on AR technique. After that, the nonlinear section model is built based on GP technique and GA is used to optimize the coefficients of the mathematic expression acquired by GP in order to obtain a more accurate model. The simulation result indicates that this hybrid model can effectively reflect the characteristics of the ASG's random drift. The square error of the ASG's random drift is reduced by 92.40%. Comparing with the AR technique and the GP + GA technique, the random drift is reduced by 9.34% and 5.06%, respectively. The hybrid modeling method can effectively compensate the ASG's random drift and improve the stability of the system.

Spin-spin interactions of electrons and also of nucleons create atomic molecular and nuclear structures

International Nuclear Information System (INIS)

Kaliambos, L.A.

2008-01-01

Fundamental interactions of spinning electrons at an interelectron separation less than 578.8 fm yield attractive electromagnetic forces with S = 0 creating vibrations under a motional emf. They explain the indistinguishability of electrons and give a vibration energy able for calculating the ground-state energies of many-electron atoms without using any perturbative approximation. Such forces create two-electron orbitals able to account for the exclusion principal and the mechanism of covalent bonds. In the outer subshells of atoms the penetrating orbitals interact also as pair-pair systems and deform drastically the probability densities of the quantum mechanical electron clouds. Such a dynamics of deformation removes the degeneracy and leads to the deviation from the shell scheme. However in the interior of atoms the large nuclear charge leads to a spherically symmetric potential with non-interacting pairs for creating shells of degenerate states giving an accurate explanation of the X-ray lines. On the other hand, considerable charge distributions in nucleons as multiples of 2e/3 and - e/3 determined by the magnetic moments, interact for creating the nuclear structure with p-n bonds. Such spin-spin interactions show that the dominant concept of the untisymmetric wave function for fermions is inapplicable not only in the simple p-n, p-p, and n-n systems but also in the LS coupling of atoms in which the electrons interact from different quantum states giving either S = 0 or S = l. (author)

Spin-Polarized Scanning Tunneling Microscope for Atomic-Scale Studies of Spin Transport, Spin Relaxation, and Magnetism in Graphene

Science.gov (United States)

2017-11-09

Polarized Scanning Tunneling Microscope for Atomic-Scale Studies of Spin Transport, Spin Relaxation, and Magnetism in Graphene Report Term: 0-Other Email ...Principal: Y Name: Jay A Gupta Email : gupta.208@osu.edu Name: Roland K Kawakami Email : kawakami.15@osu.edu RPPR Final Report as of 13-Nov-2017...studies on films and devices. Optimization of the Cr tip will be the next important step to establish this technique. We are writing up these early

Calculation of nuclear-spin-relaxation rate for spin-polarized atomic hydrogen

International Nuclear Information System (INIS)

Ahn, R.M.C.; Eijnde, J.P.H.W.V.; Verhaar, B.J.

1983-01-01

Approximations introduced in previous calculations of spin relaxation for spin-polarized atomic hydrogen are investigated by carrying out a more exact coupled-channel calculation. With the exception of the high-temperature approximation, the approximations turn out to be justified up to the 10 -3 level of accuracy. It is shown that at the lowest temperatures for which experimental data are available, the high-temperature limit underestimates relaxation rates by a factor of up to 2. For a comparison with experimental data it is also of interest to pay attention to the expression for the atomic hydrogen relaxation rates in terms of transition amplitudes for two-particle collisions. Discrepancies by a factor of 2 among previous derivations of relaxation rates are pointed out. To shed light on these discrepancies we present two alternative derivations in which special attention is paid to identical-particle aspects. Comparing with experiment, we find our theoretical volume relaxation rate to be in better agreement with measured values than that obtained by other groups. The theoretical surface relaxation rate, however, still shows a discrepancy with experiment by a factor of order 50

Nonlocally sensing the magnetic states of nanoscale antiferromagnets with an atomic spin sensor

Science.gov (United States)

Yan, Shichao; Malavolti, Luigi; Burgess, Jacob A. J.; Droghetti, Andrea; Rubio, Angel; Loth, Sebastian

2017-01-01

The ability to sense the magnetic state of individual magnetic nano-objects is a key capability for powerful applications ranging from readout of ultradense magnetic memory to the measurement of spins in complex structures with nanometer precision. Magnetic nano-objects require extremely sensitive sensors and detection methods. We create an atomic spin sensor consisting of three Fe atoms and show that it can detect nanoscale antiferromagnets through minute, surface-mediated magnetic interaction. Coupling, even to an object with no net spin and having vanishing dipolar stray field, modifies the transition matrix element between two spin states of the Fe atom–based spin sensor that changes the sensor’s spin relaxation time. The sensor can detect nanoscale antiferromagnets at up to a 3-nm distance and achieves an energy resolution of 10 μeV, surpassing the thermal limit of conventional scanning probe spectroscopy. This scheme permits simultaneous sensing of multiple antiferromagnets with a single-spin sensor integrated onto the surface. PMID:28560346

High performance current and spin diode of atomic carbon chain between transversely symmetric ribbon electrodes.

Science.gov (United States)

Dong, Yao-Jun; Wang, Xue-Feng; Yang, Shuo-Wang; Wu, Xue-Mei

2014-08-21

We demonstrate that giant current and high spin rectification ratios can be achieved in atomic carbon chain devices connected between two symmetric ferromagnetic zigzag-graphene-nanoribbon electrodes. The spin dependent transport simulation is carried out by density functional theory combined with the non-equilibrium Green's function method. It is found that the transverse symmetries of the electronic wave functions in the nanoribbons and the carbon chain are critical to the spin transport modes. In the parallel magnetization configuration of two electrodes, pure spin current is observed in both linear and nonlinear regions. However, in the antiparallel configuration, the spin-up (down) current is prohibited under the positive (negative) voltage bias, which results in a spin rectification ratio of order 10(4). When edge carbon atoms are substituted with boron atoms to suppress the edge magnetization in one of the electrodes, we obtain a diode with current rectification ratio over 10(6).

Atomic carbon chains as spin-transmitters: An ab initio transport study

DEFF Research Database (Denmark)

Fürst, Joachim Alexander; Brandbyge, Mads; Jauho, Antti-Pekka

2010-01-01

An atomic carbon chain joining two graphene flakes was recently realized in a ground-breaking experiment by Jin et al. (Phys. Rev. Lett., 102 (2009) 205501). We present ab initio results for the electron transport properties of such chains and demonstrate complete spin-polarization of the transmi......An atomic carbon chain joining two graphene flakes was recently realized in a ground-breaking experiment by Jin et al. (Phys. Rev. Lett., 102 (2009) 205501). We present ab initio results for the electron transport properties of such chains and demonstrate complete spin...

Spin-orbit coupling in ultracold Fermi gases of 173Yb atoms

Science.gov (United States)

Song, Bo; He, Chengdong; Hajiyev, Elnur; Ren, Zejian; Seo, Bojeong; Cai, Geyue; Amanov, Dovran; Zhang, Shanchao; Jo, Gyu-Boong

2017-04-01

Synthetic spin-orbit coupling (SOC) in cold atoms opens an intriguing new way to probe nontrivial topological orders beyond natural conditions. Here, we report the realization of the SOC physics both in a bulk system and in an optical lattice. First, we demonstrate two hallmarks induced from SOC in a bulk system, spin dephasing in the Rabi oscillation and asymmetric atomic distribution in the momentum space respectively. Then we describe the observation of non-trivial spin textures and the determination of the topological phase transition in a spin-dependent optical lattice dressed by the periodic Raman field. Furthermore, we discuss the quench dynamics between topological and trivial states by suddenly changing the band topology. Our work paves a new way to study non-equilibrium topological states in a controlled manner. Funded by Croucher Foundation and Research Grants Council (RGC) of Hong Kong (Project ECS26300014, GRF16300215, GRF16311516, and Croucher Innovation Grants).

Search for electric dipole moment in 129Xe atom using active nuclear spin maser

Directory of Open Access Journals (Sweden)

Ichikawa Y.

2014-03-01

Full Text Available An experimental search for an electric dipole moment in the diamagnetic atom 129Xe is in progress through the precision measurement of spin precession frequency using an active nuclear spin maser. A 3He comagnetometer has been incorporated into the active spin maser system in order to cancel out the long-term drifts in the external magnetic field. Also, a double-cell geometry has been adopted in order to suppress the frequency shifts due to interaction with polarized Rb atoms. The first EDM measurement with the 129Xe active spin maser and the 3He comagnetometer has been conducted.

Collective spin wave and phonon excitations in ferromagnetic organic polymers

International Nuclear Information System (INIS)

Leong, Jit-Liang; Sun, Shih-Jye

2013-01-01

We proposed a model to investigate the properties of a conductive and ferromagnetic organic-polymer (OCP), which contains two collective excitations—spin wave and phonon—competing with each other; namely, the spin wave excitation accompanies the electron–phonon (e–ph) interactions in the conductive and ferromagnetic OCP. The ferromagnetism of the OCP is induced from the conductive carriers which couple with the phonon to become polarons. Due to the competition between both excitations, the Curie temperature (T C ) is sensitively suppressed by the e–ph interaction. In addition, an optimal T C with a small e–ph interaction exists in a specific density of conduction carrier, yet is contrary to the large e–ph interaction case. Furthermore, the dimerization, i.e. the atomic displacement induced from the e–ph interactions, increases with the strength of the e–ph interaction and decreases upon reaching the maximum dimerization. (paper)

Spin-polarized spin excitation spectroscopy

International Nuclear Information System (INIS)

Loth, Sebastian; Lutz, Christopher P; Heinrich, Andreas J

2010-01-01

We report on the spin dependence of elastic and inelastic electron tunneling through transition metal atoms. Mn, Fe and Cu atoms were deposited onto a monolayer of Cu 2 N on Cu(100) and individually addressed with the probe tip of a scanning tunneling microscope. Electrons tunneling between the tip and the substrate exchange energy and spin angular momentum with the surface-bound magnetic atoms. The conservation of energy during the tunneling process results in a distinct onset threshold voltage above which the tunneling electrons create spin excitations in the Mn and Fe atoms. Here we show that the additional conservation of spin angular momentum leads to different cross-sections for spin excitations depending on the relative alignment of the surface spin and the spin of the tunneling electron. For this purpose, we developed a technique for measuring the same local spin with a spin-polarized and a non-spin-polarized tip by exchanging the last apex atom of the probe tip between different transition metal atoms. We derive a quantitative model describing the observed excitation cross-sections on the basis of an exchange scattering process.

Modelization of nanospace interaction involving a ferromagnetic atom: a spin polarization effect study by thermogravimetric analysis.

Science.gov (United States)

Santhanam, K S V; Chen, Xu; Gupta, S

2014-04-01

Ab initio studies of ferromagnetic atom interacting with carbon nanotubes have been reported in the literature that predict when the interaction is strong, a higher hybridization with confinement effect will result in spin polarization in the ferromagnetic atom. The spin polarization effect on the thermal oxidation to form its oxide is modeled here for the ferromagnetic atom and its alloy, as the above studies predict the 4s electrons are polarized in the atom. The four models developed here provide a pathway for distinguishing the type of interaction that exists in the real system. The extent of spin polarization in the ferromagnetic atom has been examined by varying the amount of carbon nanotubes in the composites in the thermogravimetric experiments. In this study we report the experimental results on the CoNi alloy which appears to show selective spin polarization. The products of the thermal oxidation has been analyzed by Fourier Transform Infrared Spectroscopy.

High-spin excitations of atomic nuclei

International Nuclear Information System (INIS)

Xu Furong; National Laboratory of Heavy Ion Physics, Lanzhou; Chinese Academy of Sciences, Beijing

2004-01-01

The authors used the cranking shell model to investigate the high-spin motions and structures of atomic nuclei. The authors focus the collective rotations of the A∼50, 80 and 110 nuclei. The A∼50 calculations show complicated g spectroscopy, which can have significant vibration effects. The A≅80 N≅Z nuclei show rich shape coexistence with prolate and oblate rotational bands. The A≅110 nuclei near the r-process path can have well-deformed oblate shapes that become yrast and more stable with increasing rotational frequency. As another important investigation, the authors used the configuration-constrained adiabatic method to calculate the multi-quasiparticle high-K states in the A∼130, 180 and superheavy regions. The calculations show significant shape polarizations due to quasi-particle excitations for soft nuclei, which should be considered in the investigations of high-K states. The authors predicted some important high-K isomers, e.g., the 8 - isomers in the unstable nuclei of 140 Dy and 188 Pb, which have been confirmed in experiments. In superheavy nuclei, our calculations show systematic existence of high-K states. The high-K excitations can increase the productions of synthesis and the survival probabilities of superheavy nuclei. (authors)

Spin-polarized transport properties of Fe atomic chain adsorbed on zigzag graphene nanoribbons

International Nuclear Information System (INIS)

Zhang, Z L; Chen, Y P; Xie, Y E; Zhang, M; Zhong, J X

2011-01-01

The spin-polarized transport properties of Fe atomic chain adsorbed on zigzag graphene nanoribbons (ZGNRs) are investigated using the density-functional theory in combination with the nonequilibrium Green's function method. We find that the Fe chain has drastic effects on spin-polarized transport properties of ZGNRs compared with a single Fe atom adsorbed on the ZGNRs. When the Fe chain is adsorbed on the centre of the ZGNR, the original semiconductor transforms into metal, showing a very wide range of spin-polarized transport. Particularly, the spin polarization around the Fermi level is up to 100%. This is because the adsorbed Fe chain not only induces many localized states but also has effects on the edge states of ZGNR, which can effectively modulate the spin-polarized transports. The spin polarization of ZGNRs is sensitive to the adsorption site of the Fe chain. When the Fe chain is adsorbed on the edge of ZGNR, the spin degeneracy of conductance is completely broken. The spin polarization is found to be more pronounced because the edge state of one edge is destroyed by the additional Fe chain. These results have direct implications for the control of the spin-dependent conductance in ZGNRs with the adsorption of Fe chains.

Nuclear-spin-dependent parity-nonconserving effects in thallium, lead and bismuth atoms

International Nuclear Information System (INIS)

Khriplovich, I.B.

1994-01-01

Nuclear-spin-dependent P-odd optical activity in atomic Tl, Pb and Bi is calculated. Its magnitude is expressed analytically through the main contribution to the optical rotation, which is independent of nuclear spin. The accuracy of results is discussed. 31 refs., 2 tabs

Characterization of atomic spin polarization lifetime of cesium vapor cells with neon buffer gas

Science.gov (United States)

Lou, Janet W.; Cranch, Geoffrey A.

2018-02-01

The dephasing time of spin-polarized atoms in an atomic vapor cell plays an important role in determining the stability of vapor-cell clocks as well as the sensitivity of optically-pumped magnetometers. The presence of a buffer gas can extend the lifetime of these atoms. Many vapor cell systems operate at a fixed (often elevated) temperature. For ambient temperature operation with no temperature control, it is necessary to characterize the temperature dependence as well. We present a spin-polarization lifetime study of Cesium vapor cells with different buffer gas pressures, and find good agreement with expectations based on the combined effects of wall collisions, spin exchange, and spin destruction. For our (7.5 mm diameter) vapor cells, the lifetime can be increased by two orders of magnitude by introducing Ne buffer gas up to 100 Torr. Additionally, the dependence of the lifetime on temperature is measured (25 - 47 oC) and simulated for the first time to our knowledge with reasonable agreement.

Sensing Noncollinear Magnetism at the Atomic Scale Combining Magnetic Exchange and Spin-Polarized Imaging.

Science.gov (United States)

Hauptmann, Nadine; Gerritsen, Jan W; Wegner, Daniel; Khajetoorians, Alexander A

2017-09-13

Storing and accessing information in atomic-scale magnets requires magnetic imaging techniques with single-atom resolution. Here, we show simultaneous detection of the spin-polarization and exchange force with or without the flow of current with a new method, which combines scanning tunneling microscopy and noncontact atomic force microscopy. To demonstrate the application of this new method, we characterize the prototypical nanoskyrmion lattice formed on a monolayer of Fe/Ir(111). We resolve the square magnetic lattice by employing magnetic exchange force microscopy, demonstrating its applicability to noncollinear magnetic structures for the first time. Utilizing distance-dependent force and current spectroscopy, we quantify the exchange forces in comparison to the spin-polarization. For strongly spin-polarized tips, we distinguish different signs of the exchange force that we suggest arises from a change in exchange mechanisms between the probe and a skyrmion. This new approach may enable both nonperturbative readout combined with writing by current-driven reversal of atomic-scale magnets.

Exotic pairing in 1D spin-3/2 atomic gases with SO(4 symmetry

Directory of Open Access Journals (Sweden)

Yuzhu Jiang

2015-06-01

Full Text Available Tuning interactions in the spin singlet and quintet channels of two colliding atoms could change the symmetry of the one-dimensional spin-3/2 fermionic systems of ultracold atoms while preserving the integrability. Here we find a novel SO(4 symmetry integrable point in the spin-3/2 Fermi gas and derive the exact solution of the model using the Bethe ansatz. In contrast to the model with SU(4 and SO(5 symmetries, the present model with SO(4 symmetry preserves spin singlet and quintet Cooper pairs in two sets of SU(2⊗SU(2 spin subspaces. We obtain full phase diagrams, including the Fulde–Ferrel–Larkin–Ovchinnikov like pair correlations, spin excitations and quantum criticality through the generalized Yang–Yang thermodynamic equations. In particular, various correlation functions are calculated by using finite-size corrections in the frame work of conformal field theory. Moreover, within the local density approximation, we further find that spin singlet and quintet pairs form subtle multiple shell structures in density profiles of the trapped gas.

Coupled spin and charge collective excitations in a spin polarized electron gas

International Nuclear Information System (INIS)

Marinescu, D.C.; Quinn, J.J.; Yi, K.S.

1997-01-01

The charge and longitudinal spin responses induced in a spin polarized quantum well by a weak electromagnetic field are investigated within the framework of the linear response theory. The authors evaluate the excitation frequencies for the intra- and inter-subband transitions of the collective charge and longitudinal spin density oscillations including many-body corrections beyond the random phase approximation through the spin dependent local field factors, G σ ± (q,ω). An equation-of-motion method was used to obtain these corrections in the limit of long wavelengths, and the results are given in terms of the equilibrium pair correlation function. The finite degree of spin polarization is shown to introduce coupling between the charge and spin density modes, in contrast with the result for an unpolarized system

Rapidly solidified prealloyed powders by laser spin atomization

Science.gov (United States)

Konitzer, D. G.; Walters, K. W.; Heiser, E. L.; Fraser, H. L.

1984-01-01

A new technique, termed laser spin atomization, for the production of rapidly solidified prealloyed powders is described. The results of experiments involving the production of powders of two alloys, one based on Ni, the other on Ti, are presented. The powders have been characterized using light optical metallography, scanning electron microscopy, energy dispersive X-ray spectroscopy, and Auger elec-tron spectroscopy, and these various observations are described.

Spin dynamics and Kondo physics in optical tweezers

Science.gov (United States)

Lin, Yiheng; Lester, Brian J.; Brown, Mark O.; Kaufman, Adam M.; Long, Junling; Ball, Randall J.; Isaev, Leonid; Wall, Michael L.; Rey, Ana Maria; Regal, Cindy A.

2016-05-01

We propose to use optical tweezers as a toolset for direct observation of the interplay between quantum statistics, kinetic energy and interactions, and thus implement minimum instances of the Kondo lattice model in systems with few bosonic rubidium atoms. By taking advantage of strong local exchange interactions, our ability to tune the spin-dependent potential shifts between the two wells and complete control over spin and motional degrees of freedom, we design an adiabatic tunneling scheme that efficiently creates a spin-singlet state in one well starting from two initially separated atoms (one atom per tweezer) in opposite spin state. For three atoms in a double-well, two localized in the lowest vibrational mode of each tweezer and one atom in an excited delocalized state, we plan to use similar techniques and observe resonant transfer of two-atom singlet-triplet states between the wells in the regime when the exchange coupling exceeds the mobile atom hopping. Moreover, we argue that such three-atom double-tweezers could potentially be used for quantum computation by encoding logical qubits in collective spin and motional degrees of freedom. Current address: Department of Physics, Harvard University, Cambridge, Massachusetts 02138, USA.

Shot noise as a probe of spin-correlated transport through single atoms

Science.gov (United States)

Pradhan, S.; Fransson, J.

2018-03-01

We address the shot noise in the tunneling current through a local spin, pertaining to recent experiments on magnetic adatoms and single molecular magnets. We show that both uncorrelated and spin-correlated scattering processes contribute vitally to the noise spectrum. The spin-correlated scattering processes provide an additional contribution to the Landauer-Büttiker shot noise expression, accounting for correlations between the tunneling electrons and the localized spin moment. By calculating the Fano factor, we show that both super- and sub-Poissonian shot noise can be described within our approach. Our theory provides transparent insights into noise spectroscopy, consistent with recent experiments using local probing techniques on magnetic atoms.

Design of a 1.42 GHZ spin-flip cavity for antihydrogen atoms

CERN Document Server

Caspers, F; Juhasz, B; Mahner, E; Widmann, E

2010-01-01

The ground state hyperfine transition frequency of hydrogen is known to a very high precision and therefore the measurement of this transition frequency in antihydrogen is offering one of the most accurate tests of CPT symmetry. The ASACUSA collaboration at CERN will run an experiment designed to produce ground state antihydrogen atoms in a cusp trap. These antihydrogen atoms will pass with a low rate in the order of 1 per second through a spin-flip cavity where they get excited depending on their polarization by a 1.42 GHz magnetic field. Due to the small amount of antihydrogen atoms that will be available the requirement of good field homogeneity is imposed in order to obtain an interaction with as many antihydrogen atoms as possible. This leads to a requirement of an RF field deviation of less than ±10% transverse to the beam direction over a beam aperture with 10 cm diameter. All design aspects of this new spin-flip cavity, including the required field homogeneity and vacuum aspects, are discussed.

A laser driven source of spin polarized atomic hydrogen and deuterium

International Nuclear Information System (INIS)

Poelker, M.; Coulter, K.P.; Holt, R.J.; Jones, C.E.; Kowalczyk, R.S.; Young, L.; Toporkov, D.

1993-01-01

Recent results from a laser-driven source of polarized hydrogen (H) and deuterium (D) are presented. The performance of the source is described as a function of atomic flow rate and magnetic field. The data suggest that because atomic densities in the source are high, the system can approach spin-temperature equilibrium although applied magnetic fields are much larger than the critical field of the atoms. The authors also observe that potassium contamination in the source emittance can be reduced to a negligible amount using a teflon-lined transport tube

Simultaneous production of spin-polarized ions/electrons based on two-photon ionization of laser-ablated metallic atoms

International Nuclear Information System (INIS)

Nakajima, Takashi; Yonekura, Nobuaki; Matsuo, Yukari; Kobayashi, Tohru; Fukuyama, Yoshimitsu

2003-01-01

We demonstrate the simultaneous production of spin-polarized ions/electrons using two-color, two-photon ionization of laser-ablated metallic atoms. Specifically, we have applied the developed technique to laser-ablated Sr atoms, and found that the electron-spin polarization of Sr + ions, and accordingly, the spin polarization of photoelectrons is 64%±9%, which is in good agreement with the theoretical prediction we have recently reported [T. Nakajima and N. Yonekura, J. Chem. Phys. 117, 2112 (2002)]. Our experimental results open up a simple way toward the construction of a spin-polarized dual ion/electron source

Tunable spin-orbit coupling for ultracold atoms in two-dimensional optical lattices

Science.gov (United States)

Grusdt, Fabian; Li, Tracy; Bloch, Immanuel; Demler, Eugene

2017-06-01

Spin-orbit coupling (SOC) is at the heart of many exotic band structures and can give rise to many-body states with topological order. Here we present a general scheme based on a combination of microwave driving and lattice shaking for the realization of two-dimensional SOC with ultracold atoms in systems with inversion symmetry. We show that the strengths of Rashba and Dresselhaus SOC can be independently tuned in a spin-dependent square lattice. More generally, our method can be used to open gaps between different spin states without breaking time-reversal symmetry. We demonstrate that this allows for the realization of topological insulators with nontrivial spin textures closely related to the Kane-Mele model.

Angle and Spin Resolved Auger Emission Theory and Applications to Atoms and Molecules

CERN Document Server

Lohmann, Bernd

2009-01-01

The Auger effect must be interpreted as the radiationless counterpart of photoionization and is usually described within a two-step model. Angle and spin resolved Auger emission physics deals with the theoretical and numerical description, analysis and interpretation of such types of experiments on free atoms and molecules. This monograph derives the general theory applying the density matrix formalism and, in terms of irreducible tensorial sets, so called state multipoles and order parameters, for parameterizing the atomic and molecular systems, respectively. Propensity rules and non-linear dependencies between the angular distribution and spin polarization parameters are included in the discussion. The numerical approaches utilizing relativistic distorted wave (RDWA), multiconfigurational Dirac-Fock (MCDF), and Greens operator methods are described. These methods are discussed and applied to theoretical predictions, numerical results and experimental data for a variety of atomic systems, especially the rare...

Collective spin by linearization of the Schrodinger equation for nuclear collective motion

International Nuclear Information System (INIS)

Greiner, M.; Scheid, W.; Herrmann, R.

1988-01-01

The free Schrodinger equation for multipole degrees of freedom is linearized so that energy and momentum operators appear only in first order. As an example, the authors demonstrate the linearization procedure for quadrupole degrees of freedom. The wave function solving this equation carries a spin. The authors derive the operator of the collective spin and its eigen values depending on multipolarity

Polarization of stable and radioactive noble gas nuclei by spin exchange with laser pumped alkali atoms

International Nuclear Information System (INIS)

Calaprice, F.; Happer, W.; Schreiber, D.

1984-01-01

The nuclei of noble gases can be strongly polarized by spin exchange with sufficiently dense optically pumped alkali vapors. Only a small fraction of the spin angular momentum of the alkali atoms is transferred to the nuclear spin of the noble gas. Most of the spin angular momentum is lost to translational angular momentum of the alkali and noble gas atoms about each other. For heavy noble gases most of the angular momentum transfer occurs in alkali-noble-gas van der Waals molecules. The transfer efficiency depends on the formation and breakup rates of the van der Waals molecules in the ambient gas. Experimental methods to measure the spin transfer efficiencies have been developed. Nuclei of radioactive noble gases have been polarized by these methods, and the polarization has been detected by observing the anisotropy of the radioactive decay products. Very precise measurements of the magnetic moments of the radioactive nuclei have been made. 12 references, 9 figures

Magnetism, Spin Texture, and In-Gap States: Atomic Specialization at the Surface of Oxygen-Deficient SrTiO_{3}.

Science.gov (United States)

Altmeyer, Michaela; Jeschke, Harald O; Hijano-Cubelos, Oliver; Martins, Cyril; Lechermann, Frank; Koepernik, Klaus; Santander-Syro, Andrés F; Rozenberg, Marcelo J; Valentí, Roser; Gabay, Marc

2016-04-15

Motivated by recent spin- and angular-resolved photoemission (SARPES) measurements of the two-dimensional electronic states confined near the (001) surface of oxygen-deficient SrTiO_{3}, we explore their spin structure by means of ab initio density functional theory (DFT) calculations of slabs. Relativistic nonmagnetic DFT calculations display Rashba-like spin winding with a splitting of a few meV and when surface magnetism on the Ti ions is included, bands become spin-split with an energy difference ∼100  meV at the Γ point, consistent with SARPES findings. While magnetism tends to suppress the effects of the relativistic Rashba interaction, signatures of it are still clearly visible in terms of complex spin textures. Furthermore, we observe an atomic specialization phenomenon, namely, two types of electronic contributions: one is from Ti atoms neighboring the oxygen vacancies that acquire rather large magnetic moments and mostly create in-gap states; another comes from the partly polarized t_{2g} itinerant electrons of Ti atoms lying further away from the oxygen vacancy, which form the two-dimensional electron system and are responsible for the Rashba spin winding and the spin splitting at the Fermi surface.

Coherent storage of temporally multimode light using a spin-wave atomic frequency comb memory

International Nuclear Information System (INIS)

Gündoğan, M; Mazzera, M; Ledingham, P M; Cristiani, M; De Riedmatten, H

2013-01-01

We report on the coherent and multi-temporal mode storage of light using the full atomic frequency comb memory scheme. The scheme involves the transfer of optical atomic excitations in Pr 3+ :Y 2 SiO 5 to spin waves in hyperfine levels using strong single-frequency transfer pulses. Using this scheme, a total of five temporal modes are stored and recalled on-demand from the memory. The coherence of the storage and retrieval is characterized using a time-bin interference measurement resulting in visibilities higher than 80%, independent of the storage time. This coherent and multimode spin-wave memory is promising as a quantum memory for light. (paper)

Collective motion with anticipation: flocking, spinning, and swarming.

Science.gov (United States)

Morin, Alexandre; Caussin, Jean-Baptiste; Eloy, Christophe; Bartolo, Denis

2015-01-01

We investigate the collective dynamics of self-propelled particles able to probe and anticipate the orientation of their neighbors. We show that a simple anticipation strategy hinders the emergence of homogeneous flocking patterns. Yet anticipation promotes two other forms of self-organization: collective spinning and swarming. In the spinning phase, all particles follow synchronous circular orbits, while in the swarming phase, the population condensates into a single compact swarm that cruises coherently without requiring any cohesive interactions. We quantitatively characterize and rationalize these phases of polar active matter and discuss potential applications to the design of swarming robots.

Non-thermalization in trapped atomic ion spin chains

Science.gov (United States)

Hess, P. W.; Becker, P.; Kaplan, H. B.; Kyprianidis, A.; Lee, A. C.; Neyenhuis, B.; Pagano, G.; Richerme, P.; Senko, C.; Smith, J.; Tan, W. L.; Zhang, J.; Monroe, C.

2017-10-01

Linear arrays of trapped and laser-cooled atomic ions are a versatile platform for studying strongly interacting many-body quantum systems. Effective spins are encoded in long-lived electronic levels of each ion and made to interact through laser-mediated optical dipole forces. The advantages of experiments with cold trapped ions, including high spatio-temporal resolution, decoupling from the external environment and control over the system Hamiltonian, are used to measure quantum effects not always accessible in natural condensed matter samples. In this review, we highlight recent work using trapped ions to explore a variety of non-ergodic phenomena in long-range interacting spin models, effects that are heralded by the memory of out-of-equilibrium initial conditions. We observe long-lived memory in static magnetizations for quenched many-body localization and prethermalization, while memory is preserved in the periodic oscillations of a driven discrete time crystal state. This article is part of the themed issue 'Breakdown of ergodicity in quantum systems: from solids to synthetic matter'.

Silver atom solvation and desolvation in ice matrices: study of solvation shell geometry by electron spin resonance and electron spin echo methods

Energy Technology Data Exchange (ETDEWEB)

Kevan, L; Narayana, P A

1978-01-01

Results of studies of the solvation shell structure of silver atoms in ice matrix at 4/sup 0/K by electron spin resonance (ESR) and electron spin echo spectrometry are reported. Drastic change in the hyperfine coupling constant of the silver atom was noted when the silver atom initially produced at 4/sup 0/K was warmed to 77/sup 0/K and reexamined by ESR at 4/sup 0/K. This suggested a very drastic rearrangement of the water molecules surrounding the silver atom. The geometric arrangement of water molecules around the silver atom produced at 4/sup 0/K was what would be expected for a solvated silver ion, indicating that no rearrangement had occurred after the silver atom formed. The addition of a little thermal excitation (heating to 77/sup 0/K) results in the geometry changes than can be explained by assuming either that a water molecule rotates around one of its OH bands or by the development of a hydrogen bond between the silver atom and one of the first solvation shell water molecules. Optical excitation in the absorption band of the silver atom in the ice matrix at 400nm resulted in desolvation of the silver ion or a reversion to the structure originally obtained by reaction of solver salts in ic matrix with radiation produced electrons. This was best explained by a charge transfer mechanism. (BLM)

Measurement of atomic-hydrogen spin-exchange parameters at 0.5 K using a cryogenic hydrogen maser

International Nuclear Information System (INIS)

Hayden, M.E.; Huerlimann, M.D.; Hardy, W.N.

1996-01-01

Using a cryogenic hydrogen maser, suitably modified to have electronic control of both the resonance frequency and the quality factor of the external cavity, we have measured a number of spin-exchange parameters for an atomic-hydrogen (H) gas at a temperature of 0.5 K. These results are relevant to the ultimate achievable frequency stability for cryogenic H masers and, when coupled with accurate calculations of the spin-exchange parameters, serve as a sensitive test of the H-H interatomic potentials. We find evidence for a frequency shift not predicted by semiclassical theories of spin exchange. In the context of a fully quantum mechanical hydrogen-atom spin-exchange theory [B. J. Verhaar et al., Phys. Rev. A 35, 3825 (1987) and J. M. V. A. Koelman et al., Phys. Rev. A 38, 3535 (1988)], this frequency shift is attributed to the influence of hyperfine interactions during spin-exchange collisions. Our findings are generally in agreement with these predictions; however, the sign of the hyperfine-induced frequency shift appears to differ from theory. copyright 1996 The American Physical Society

Realistic Rashba and Dresselhaus spin-orbit coupling for neutral atoms

International Nuclear Information System (INIS)

Campbell, D. L.; Spielman, I. B.; Juzeliunas, G.

2011-01-01

We describe a new class of atom-laser coupling schemes which lead to spin-orbit-coupled Hamiltonians for ultracold neutral atoms. By properly setting the optical phases, a pair of degenerate pseudospin (a linear combination of internal atomic) states emerge as the lowest-energy eigenstates in the spectrum and are thus immune to collisionally induced decay. These schemes use N cyclically coupled ground or metastable internal states. We focus on two situations: a three-level case and a four-level case, where the latter adds a controllable Dresselhaus contribution. We describe an implementation of the four-level scheme for 87 Rb and analyze its sensitivity to typical laboratory noise sources. Last, we argue that the Rashba Hamiltonian applies only in the large intensity limit since any laser coupling scheme will produce terms nonlinear in momentum that decline with intensity.

Nuclear spin content and constraints on exotic spin-dependent couplings

International Nuclear Information System (INIS)

Kimball, D F Jackson

2015-01-01

There are numerous recent and ongoing experiments employing a variety of atomic species to search for couplings of atomic spins to exotic fields. In order to meaningfully compare these experimental results, the coupling of the exotic field to the atomic spin must be interpreted in terms of the coupling to electron, proton, and neutron spins. Traditionally, constraints from atomic experiments on exotic couplings to neutron and proton spins have been derived using the single-particle Schmidt model for nuclear spin. In this model, particular atomic species are sensitive to either neutron or proton spin couplings, but not both. More recently, semi-empirical models employing nuclear magnetic moment data have been used to derive new constraints for non-valence nucleons. However, comparison of such semi-empirical models to detailed large-scale nuclear shell model calculations and analysis of known physical effects in nuclei show that existing semi-empirical models cannot reliably be used to predict the spin polarization of non-valence nucleons. The results of our re-analysis of nuclear spin content are applied to searches for exotic long-range monopole–dipole and dipole–dipole couplings of nuclei leading to significant revisions of some published constraints. (paper)

Application of the Ursell-Mayer method in the theory of spin-polarized atomic hydrogen

International Nuclear Information System (INIS)

Kilic, S.; Radelja, T.

1981-01-01

Employing the Ursell-Mayer method and Ljolje semi-free gas model analytic relations describing ground state properties (energy, pressure, compressibility, sound velocity, radial distribution function and one-particle density matrix) of spin-polarized atomic hydrogen were derived. The expressions are valid up to density 2 10 26 atoms/m 3 . It was found out that at density of 2 10 26 atoms/m 3 the condensation of particle in momentum space is 88% (at absolute zero). (orig.)

Methods for Computing Accurate Atomic Spin Moments for Collinear and Noncollinear Magnetism in Periodic and Nonperiodic Materials.

Science.gov (United States)

Manz, Thomas A; Sholl, David S

2011-12-13

The partitioning of electron spin density among atoms in a material gives atomic spin moments (ASMs), which are important for understanding magnetic properties. We compare ASMs computed using different population analysis methods and introduce a method for computing density derived electrostatic and chemical (DDEC) ASMs. Bader and DDEC ASMs can be computed for periodic and nonperiodic materials with either collinear or noncollinear magnetism, while natural population analysis (NPA) ASMs can be computed for nonperiodic materials with collinear magnetism. Our results show Bader, DDEC, and (where applicable) NPA methods give similar ASMs, but different net atomic charges. Because they are optimized to reproduce both the magnetic field and the chemical states of atoms in a material, DDEC ASMs are especially suitable for constructing interaction potentials for atomistic simulations. We describe the computation of accurate ASMs for (a) a variety of systems using collinear and noncollinear spin DFT, (b) highly correlated materials (e.g., magnetite) using DFT+U, and (c) various spin states of ozone using coupled cluster expansions. The computed ASMs are in good agreement with available experimental results for a variety of periodic and nonperiodic materials. Examples considered include the antiferromagnetic metal organic framework Cu3(BTC)2, several ozone spin states, mono- and binuclear transition metal complexes, ferri- and ferro-magnetic solids (e.g., Fe3O4, Fe3Si), and simple molecular systems. We briefly discuss the theory of exchange-correlation functionals for studying noncollinear magnetism. A method for finding the ground state of systems with highly noncollinear magnetism is introduced. We use these methods to study the spin-orbit coupling potential energy surface of the single molecule magnet Fe4C40H52N4O12, which has highly noncollinear magnetism, and find that it contains unusual features that give a new interpretation to experimental data.

Nuclear spin polarized H and D by means of spin-exchange optical pumping

Science.gov (United States)

Stenger, Jörn; Grosshauser, Carsten; Kilian, Wolfgang; Nagengast, Wolfgang; Ranzenberger, Bernd; Rith, Klaus; Schmidt, Frank

1998-01-01

Optically pumped spin-exchange sources for polarized hydrogen and deuterium atoms have been demonstrated to yield high atomic flow and high electron spin polarization. For maximum nuclear polarization the source has to be operated in spin temperature equilibrium, which has already been demonstrated for hydrogen. In spin temperature equilibrium the nuclear spin polarization PI equals the electron spin polarization PS for hydrogen and is even larger than PS for deuterium. We discuss the general properties of spin temperature equilibrium for a sample of deuterium atoms. One result are the equations PI=4PS/(3+PS2) and Pzz=PSṡPI, where Pzz is the nuclear tensor polarization. Furthermore we demonstrate that the deuterium atoms from our source are in spin temperature equilibrium within the experimental accuracy.

Spin-polarized hydrogen Rydberg time-of-flight: Experimental measurement of the velocity-dependent H atom spin-polarization

International Nuclear Information System (INIS)

Broderick, Bernadette M.; Lee, Yumin; Doyle, Michael B.; Chernyak, Vladimir Y.; Suits, Arthur G.; Vasyutinskii, Oleg S.

2014-01-01

We have developed a new experimental method allowing direct detection of the velocity dependent spin-polarization of hydrogen atoms produced in photodissociation. The technique, which is a variation on the H atom Rydberg time-of-flight method, employs a double-resonance excitation scheme and experimental geometry that yields the two coherent orientation parameters as a function of recoil speed for scattering perpendicular to the laser propagation direction. The approach, apparatus, and optical layout we employ are described here in detail and demonstrated in application to HBr and DBr photolysis at 213 nm. We also discuss the theoretical foundation for the approach, as well as the resolution and sensitivity we achieve

Linear spin waves in a trapped Bose gas

International Nuclear Information System (INIS)

Nikuni, T.; Williams, J.E.; Clark, C.W.

2002-01-01

An ultracold Bose gas of two-level atoms can be thought of as a spin-1/2 Bose gas. It supports spin-wave collective modes due to the exchange mean field. Such collective spin oscillations have been observed in recent experiments at JILA with 87 Rb atoms confined in a harmonic trap. We present a theory of the spin-wave collective modes based on the moment method for trapped gases. In the collisionless and hydrodynamic limits, we derive analytic expressions for the frequencies and damping rates of modes with dipole and quadrupole symmetry. We find that the frequency for a given mode is given by a temperature-independent function of the peak density n, and falls off as 1/n. We also find that, to a very good approximation, excitations in the radial and axial directions are decoupled. We compare our model to the numerical integration of a one-dimensional version of the kinetic equation and find very good qualitative agreement. The damping rates, however, show the largest deviation for intermediate densities, where one expects Landau damping--which is unaccounted for in our moment approach--to play a significant role

Observation of Spin-Polarons in a strongly interacting Fermi liquid

Science.gov (United States)

Zwierlein, Martin

2009-03-01

We have observed spin-polarons in a highly imbalanced mixture of fermionic atoms using tomographic RF spectroscopy. Feshbach resonances allow to freely tune the interactions between the two spin states involved. A single spin down atom immersed in a Fermi sea of spin up atoms can do one of two things: For strong attraction, it can form a molecule with exactly one spin up partner, but for weaker interaction it will spread its attraction and surround itself with a collection of majority atoms. This spin down atom ``dressed'' with a spin up cloud constitutes the spin-polaron. We have observed a striking spectroscopic signature of this quasi-particle for various interaction strengths, a narrow peak in the spin down spectrum that emerges above a broad background. The narrow width signals a long lifetime of the spin-polaron, much longer than the collision rate with spin up atoms, as it must be for a proper quasi-particle. The peak position allows to directly measure the polaron energy. The broad pedestal at high energies reveals physics at short distances and is thus ``molecule-like'': It is exactly matched by the spin up spectra. The comparison with the area under the polaron peak allows to directly obtain the quasi-particle weight Z. We observe a smooth transition from polarons to molecules. At a critical interaction strength of 1/kFa = 0.7, the polaron peak vanishes and spin up and spin down spectra exactly match, signalling the formation of molecules. This is the same critical interaction strength found earlier to separate a normal Fermi mixture from a superfluid molecular Bose-Einstein condensate. The spin-polarons determine the low-temperature phase diagram of imbalanced Fermi mixtures. In principle, polarons can interact with each other and should, at low enough temperatures, form a superfluid of p-wave pairs. We will present a first indication for interactions between polarons.

Accurate Mapping of Multilevel Rydberg Atoms on Interacting Spin-1 /2 Particles for the Quantum Simulation of Ising Models

Science.gov (United States)

de Léséleuc, Sylvain; Weber, Sebastian; Lienhard, Vincent; Barredo, Daniel; Büchler, Hans Peter; Lahaye, Thierry; Browaeys, Antoine

2018-03-01

We study a system of atoms that are laser driven to n D3 /2 Rydberg states and assess how accurately they can be mapped onto spin-1 /2 particles for the quantum simulation of anisotropic Ising magnets. Using nonperturbative calculations of the pair potentials between two atoms in the presence of electric and magnetic fields, we emphasize the importance of a careful selection of experimental parameters in order to maintain the Rydberg blockade and avoid excitation of unwanted Rydberg states. We benchmark these theoretical observations against experiments using two atoms. Finally, we show that in these conditions, the experimental dynamics observed after a quench is in good agreement with numerical simulations of spin-1 /2 Ising models in systems with up to 49 spins, for which numerical simulations become intractable.

Effects of disorder on atomic density waves and spin-singlet dimers in one-dimensional optical lattices

International Nuclear Information System (INIS)

Gao Xianlong

2008-01-01

Using the Bethe-ansatz density-functional theory, we study a one-dimensional Hubbard model of confined attractively interacting fermions in the presence of a uniformly distributed disorder. The strongly correlated Luther-Emery nature of the attractive one-dimensional Hubbard model is fully taken into account as the reference system in the density-functional theory. The effects of the disorder are investigated on the atomic density waves in the weak-to-intermediate attractive interaction and on the spin-singlet dimers of doubly occupied sites in the strongly attractive regime. It is found that atomic density waves are sensitive to the disorder and the spin-singlet dimers of doubly occupied sites are quite unstable against the disorder. We also show that a very weak disorder could smear the singularities in the stiffness, thus, suppresses the spin-singlet pairs

Relativistic Spin-Orbit Heavy Atom on the Light Atom NMR Chemical Shifts: General Trends Across the Periodic Table Explained.

Science.gov (United States)

Vícha, Jan; Komorovsky, Stanislav; Repisky, Michal; Marek, Radek; Straka, Michal

2018-05-10

The importance of relativistic effects on the NMR parameters in heavy-atom (HA) compounds, particularly the SO-HALA (Spin-Orbit Heavy Atom on the Light Atom) effect on NMR chemical shifts, has been known for about 40 years. Yet, a general correlation between the electronic structure and SO-HALA effect has been missing. By analyzing 1 H NMR chemical shifts of the sixth-period hydrides (Cs-At), we discovered general electronic-structure principles and mechanisms that dictate the size and sign of the SO-HALA NMR chemical shifts. In brief, partially occupied HA valence shells induce relativistic shielding at the light atom (LA) nuclei, while empty HA valence shells induce relativistic deshielding. In particular, the LA nucleus is relativistically shielded in 5d 2 -5d 8 and 6p 4 HA hydrides and deshielded in 4f 0 , 5d 0 , 6s 0 , and 6p 0 HA hydrides. This general and intuitive concept explains periodic trends in the 1 H NMR chemical shifts along the sixth-period hydrides (Cs-At) studied in this work. We present substantial evidence that the introduced principles have a general validity across the periodic table and can be extended to nonhydride LAs. The decades-old question of why compounds with occupied frontier π molecular orbitals (MOs) cause SO-HALA shielding at the LA nuclei, while the frontier σ MOs cause deshielding is answered. We further derive connection between the SO-HALA NMR chemical shifts and Spin-Orbit-induced Electron Deformation Density (SO-EDD), a property that can be obtained easily from differential electron densities and can be represented graphically. SO-EDD provides an intuitive understanding of the SO-HALA effect in terms of the depletion/concentration of the electron density at LA nuclei caused by spin-orbit coupling due to HA in the presence of a magnetic field. Using an analogy between the SO-EDD concept and arguments from classic NMR theory, the complex question of the SO-HALA NMR chemical shifts becomes easily understandable for a wide

Tunable self-assembled spin chains of strongly interacting cold atoms for demonstration of reliable quantum state transfer

DEFF Research Database (Denmark)

Loft, N. J. S.; Marchukov, O. V.; Petrosyan, D.

2016-01-01

We have developed an efficient computational method to treat long, one-dimensional systems of strongly-interacting atoms forming self-assembled spin chains. Such systems can be used to realize many spin chain model Hamiltonians tunable by the external confining potential. As a concrete...... demonstration, we consider quantum state transfer in a Heisenberg spin chain and we show how to determine the confining potential in order to obtain nearly-perfect state transfer....

Emerging bosons with three-body interactions from spin-1 atoms in optical lattices

International Nuclear Information System (INIS)

Mazza, L.; Rizzi, M.; Cirac, J. I.; Lewenstein, M.

2010-01-01

We study two many-body systems of bosons interacting via an infinite three-body contact repulsion in a lattice: a pairs quasicondensate induced by correlated hopping and the discrete version of the Pfaffian wave function. We propose to experimentally realize systems characterized by such interaction by means of a proper spin-1 lattice Hamiltonian: spin degrees of freedom are locally mapped into occupation numbers of emerging bosons, in a fashion similar to spin-1/2 and hardcore bosons. Such a system can be realized with ultracold spin-1 atoms in a Mott insulator with a filling factor of 1. The high versatility of these setups allows us to engineer spin-hopping operators breaking the SU(2) symmetry, as needed to approximate interesting bosonic Hamiltonians with three-body hardcore constraint. For this purpose we combine bichromatic spin-independent superlattices and Raman transitions to induce a different hopping rate for each spin orientation. Finally, we illustrate how our setup could be used to experimentally realize the first setup, that is, the transition to a pairs quasicondensed phase of the emerging bosons. We also report on a route toward the realization of a discrete bosonic Pfaffian wave function and list some open problems for reaching this goal.

Frequency Fine-tuning of a Spin-flip Cavity for Antihydrogen Atoms

CERN Document Server

Federmann, S; Mahner, E; Juhasz, B; Widmann, E

2012-01-01

As part of the ASACUSA (Atomic Spectroscopy And Collisions Using Slow Antiprotons) physics program a spin-flip cavity, for measurements of the ground-state hyperfine transition frequency of antihydrogen atoms, is needed. The purpose of the cavity is to excite antihydrogen atoms depending on their polarisation by a microwave field operating at 1.42 GHz. The delicacy of designing such a cavity lies in achieving and maintaining the required properties of this field over a large aperture of 10 cm and for a long period of time (required amplitude stability is 1% over 12 h). This paper presents the frequency fine tuning techniques developed to obtain the desired centre frequency of 1.42GHz with a Q value below 500 as well as the circuit used for the frequency sweep over a bandwidth of 6MHz.

Theory of longitudinal atomic beam spin echo and parity violating Berry-phases in atoms; Theorie des longitudinalen Atomstrahl-Spinechos und paritaetsverletzende Berry-Phasen in Atomen

Energy Technology Data Exchange (ETDEWEB)

Bergmann, T.F.

2006-07-19

We present a nonrelativistic theory for the quantum mechanical description of longitudinal atomic beam spin echo experiments, where a beam of neutral atoms is subjected to static electric and magnetic fields. The atomic wave function is the solution of a matrix-valued Schroedinger equation and can be written as superposition of local (atomic) eigenstates of the potential matrix. The position- and time-dependent amplitude function of each eigenstate represents an atomic wave packet and can be calculated in a series expansion with a master formula that we derive. The zeroth order of this series expansion describes the adiabatic limit, whereas the higher order contributions contain the mixing of the eigenstates and the corresponding amplitude functions. We give a tutorial for the theoretical description of longitudinal atomic beam spin echo experiments and for the so-called Fahrplan model, which is a visualisation tool for the propagation of wave packets of different atomic eigenstates. As an example for the application of our theory, we study parity violating geometric (Berry-)phases. In this context, we define geometric flux densities, which for certain field configurations can be used to illustrate geometric phases in a vector diagram. Considering an example with a specific field configuration, we prove the existence of a parity violating geometric phase. (orig.)

Force on an electric/magnetic dipole and classical approach to spin-orbit coupling in hydrogen-like atoms

Science.gov (United States)

Kholmetskii, A. L.; Missevitch, O. V.; Yarman, T.

2017-09-01

We carry out the classical analysis of spin-orbit coupling in hydrogen-like atoms, using the modern expressions for the force and energy of an electric/magnetic dipole in an electromagnetic field. We disclose a novel physical meaning of this effect and show that for a laboratory observer the energy of spin-orbit interaction is represented solely by the mechanical energy of the spinning electron (considered as a gyroscope) due to the Thomas precession of its spin. Concurrently we disclose some errors in the old and new publications on this subject.

Circuit-quantum electrodynamics with direct magnetic coupling to single-atom spin qubits in isotopically enriched 28Si

Directory of Open Access Journals (Sweden)

Guilherme Tosi

2014-08-01

Full Text Available Recent advances in silicon nanofabrication have allowed the manipulation of spin qubits that are extremely isolated from noise sources, being therefore the semiconductor equivalent of single atoms in vacuum. We investigate the possibility of directly coupling an electron spin qubit to a superconducting resonator magnetic vacuum field. By using resonators modified to increase the vacuum magnetic field at the qubit location, and isotopically purified 28Si substrates, it is possible to achieve coupling rates faster than the single spin dephasing. This opens up new avenues for circuit-quantum electrodynamics with spins, and provides a pathway for dispersive read-out of spin qubits via superconducting resonators.

Study of apical oxygen atoms in a spin-ladder cuprate compound by X-ray absorption spectroscopy near the Cu K edge

Energy Technology Data Exchange (ETDEWEB)

Hatterer, C.J.; Eustache, B.; Collin, L.; Beuran, C.F.; Partiot, C.; Germain, P.; Xu, X.Z.; Lagues, M. [CNRS, Paris (France). Surfaces et Supraconducteurs; Michalowicz, A. [Laboratoire de Physique des Milieux Desordonnes, Universite Paris XII Val-de-Marne, 61 avenue du general de Gaulle, 94010, Creteil Cedex (France)]|[LURE, Universite Paris Sud, 91405, Orsay Cedex (France); Moscovici, J. [Laboratoire de Physique des Milieux Desordonnes, Universite Paris XII Val-de-Marne, 61 avenue du general de Gaulle, 94010, Creteil Cedex (France); Deville Cavellin, C. [CNRS, Paris (France). Surfaces et Supraconducteurs]|[Laboratoire d`Electronique, Universite Paris XII Val-de-Marne, 61 av. du general de Gaulle, 94010, Creteil Cedex (France); Traverse, A. [LURE, Universite Paris Sud, 91405, Orsay Cedex (France)

1997-04-01

The structure of high-T{sub c} superconducting cuprate compounds is based on CuO{sub 2} planes alternating with blocks that behave as charge reservoirs. The apical oxygen atoms which belong to these reservoirs are suspected to play a role in the mechanism of superconductivity. It thus seems necessary to measure the amount of apical oxygen atoms in various compounds, as a function of the superconducting properties. Polarisation dependent X-ray absorption spectroscopy (XAS) measurements were performed near the Cu K-edge on three types of phases. We collected information about the neighbourhood of the copper atom in the cuprate planes and in the direction perpendicular to these planes. Two of these phases have well known structures: Bi2212 in which copper atoms are on a pyramidal site and infinite layer phase, a square planar cuprate without apical oxygen. We used the obtained results as reference data to study a new copper-rich phase related to the spin-ladder series. (orig.)

First-Order Quantum Phase Transition for Dicke Model Induced by Atom-Atom Interaction

International Nuclear Information System (INIS)

Zhao Xiu-Qin; Liu Ni; Liang Jiu-Qing

2017-01-01

In this article, we use the spin coherent state transformation and the ground state variational method to theoretically calculate the ground function. In order to consider the influence of the atom-atom interaction on the extended Dicke model’s ground state properties, the mean photon number, the scaled atomic population and the average ground energy are displayed. Using the self-consistent field theory to solve the atom-atom interaction, we discover the system undergoes a first-order quantum phase transition from the normal phase to the superradiant phase, but a famous Dicke-type second-order quantum phase transition without the atom-atom interaction. Meanwhile, the atom-atom interaction makes the phase transition point shift to the lower atom-photon collective coupling strength. (paper)

Observation of ESR spin flip satellite lines of trapped hydrogen atoms in solid H2 at 4.2 K

International Nuclear Information System (INIS)

Miyazaki, Tetsuo; Iwata, Nobuchika; Fueki, Kenji; Hase, Hirotomo

1990-01-01

ESR spectra of H atoms, produced in γ-irradiated solid H 2 , were studied at 4.2 K. Two main lines of the ESR spectra of H atoms that are separated by about 500 G accompanied two weak satellite lines. Both satellite lines and main lines decrease with the same decay rate. In the D 2 -H 2 mixtures, the satellite-line intensity depends upon the number of matrix protons. The spacing of the satellites from the main lines is equal to that of the NMR proton resonance frequency. It was concluded that the satellite lines were not ascribable to paired atoms but to spin flip lines due to an interaction of H atoms with matrix protons. The analysis of the spin flip lines and the main lines suggests that H atoms in solid H 2 are trapped in the substitutional site

Measure synchronization in a spin-orbit-coupled bosonic Josephson junction

Science.gov (United States)

Wang, Wen-Yuan; Liu, Jie; Fu, Li-Bin

2015-11-01

We present measure synchronization (MS) in a bosonic Josephson junction with spin-orbit coupling. The two atomic hyperfine states are coupled by a Raman dressing scheme, and they are regarded as two orientations of a pseudo-spin-1 /2 system. A feature specific to a spin-orbit-coupled (SOC) bosonic Josephson junction is that the transition from non-MS to MS dynamics can be modulated by Raman laser intensity, even in the absence of interspin atomic interaction. A phase diagram of non-MS and MS dynamics as functions of Raman laser intensity and Josephson tunneling amplitude is presented. Taking into account interspin atomic interactions, the system exhibits MS breaking dynamics resulting from the competition between intraspin and interspin atomic interactions. When interspin atomic interactions dominate in the competition, the system always exhibits MS dynamics. For interspin interaction weaker than intraspin interaction, a window for non-MS dynamics is present. Since SOC Bose-Einstein condensates provide a powerful platform for studies on physical problems in various fields, the study of MS dynamics is valuable in researching the collective coherent dynamical behavior in a spin-orbit-coupled bosonic Josephson junction.

Electron ionization and spin polarization control of Fe atom adsorbed graphene irradiated by a femtosecond laser

International Nuclear Information System (INIS)

Yu, Dong; Jiang, Lan; Wang, Feng; Li, Xin; Qu, Liangti; Lu, Yongfeng

2015-01-01

We investigate the structural properties and ionized spin electrons of an Fe–graphene system, in which the time-dependent density functional theory (TDDFT) within the generalized gradient approximation is used. The electron dynamics, including electron ionization and ionized electron spin polarization, is described for Fe atom adsorbed graphene under femtosecond laser irradiation. The theoretical results show that the electron ionization and ionized electron spin polarization are sensitive to the laser parameters, such as the incident angle and the peak intensity. The spin polarization presents the maximum value under certain laser parameters, which may be used as a source of spin-polarized electrons. - Highlights: • The structural properties of Fe–graphene system are investigated. • The electron dynamics of Fe–graphene system under laser irradiation are described. • The Fe–graphene system may be used as a source of spin-polarized electrons

Rényi Entropies from Random Quenches in Atomic Hubbard and Spin Models

Science.gov (United States)

Elben, A.; Vermersch, B.; Dalmonte, M.; Cirac, J. I.; Zoller, P.

2018-02-01

We present a scheme for measuring Rényi entropies in generic atomic Hubbard and spin models using single copies of a quantum state and for partitions in arbitrary spatial dimensions. Our approach is based on the generation of random unitaries from random quenches, implemented using engineered time-dependent disorder potentials, and standard projective measurements, as realized by quantum gas microscopes. By analyzing the properties of the generated unitaries and the role of statistical errors, with respect to the size of the partition, we show that the protocol can be realized in existing quantum simulators and used to measure, for instance, area law scaling of entanglement in two-dimensional spin models or the entanglement growth in many-body localized systems.

Collective and planetary motion in atoms

International Nuclear Information System (INIS)

Berry, R.S.

1986-01-01

The evolution of the conception of electron correlation is sketched, particularly the ideas that emerged in the late 1970s. Those ideas have led to a deep reexamination of the behavior of electrons sharing a valence shell. Doubly-excited helium was the first case in which it could be clearly established that the electronic states exhibit collective rotations and vibrations, rather than predominantly independent-particle-like behavior. More recently, it has appeared that the ground states and most but not all of the low-lying excited states of the alkaline-earth atoms are also much more like collective rotor-vibrators than like quantum analogues of solar systems. The appearance of such molecule-like characteristics for the electrons in atoms leads to a search for independent-particle-like behavior for atoms in highly excited vibrational states of small molecules such as H 2 O, NH 3 and CH 4 . Together, the two kinds of systems potentially exhibiting characteristics traditionally associated with the other suggest trying to find a more unified formulation of few-body problems that makes collective and independent-particle behavior into related but complementary manifestations of some more general characterization of the states of few-body systems. (Auth.)

Calculations with the quasirelativistic local-spin-density-functional theory for high-Z atoms

International Nuclear Information System (INIS)

Guo, Y.; Whitehead, M.A.

1988-01-01

The generalized-exchange local-spin-density-functional theory (LSD-GX) with relativistic corrections of the mass velocity and Darwin terms has been used to calculate statistical total energies for the neutral atoms, the positive ions, and the negative ions for high-Z elements. The effect of the correlation and relaxation correction on the statistical total energy is discussed. Comparing the calculated results for the ionization potentials and electron affinities for the atoms (atomic number Z from 37 to 56 and 72 to 80) with experiment, shows that for the atoms rubidium to barium both the LSD-GX and the quasirelativistic LSD-GX, with self-interaction correction, Gopinathan, Whitehead, and Bogdanovic's Fermi-hole parameters [Phys. Rev. A 14, 1 (1976)], and Vosko, Wilk, and Nusair's correlation correction [Can. J. Phys. 58, 1200 (1980)], are very good methods for calculating ionization potentials and electron affinities. For the atoms hafnium to mercury the relativistic effect has to be considered

Differential saturation study of radial and angular modulation mechanisms of electron spin--lattice relaxation for trapped hydrogen atoms in sulfuric acid glasses. [X radiation

Energy Technology Data Exchange (ETDEWEB)

Plonka, A; Kevan, L

1976-11-01

A differential ESR saturation study of allowed transitions and forbidden proton spin-flip satellite transitions for trapped hydrogen atoms in sulfuric acid glasses indicates that angular modulation dominates the spin-lattice relaxation mechanisms and suggests that the modulation arises from motion of the H atom.

Nanocluster formation by spin coating : quantitative atomic force microscopy and Rutherford backscattering spectrometry analysis

NARCIS (Netherlands)

Partridge, A.; Toussaint, S.L.G.; Flipse, C.F.J.; IJzendoorn, van L.J.; Oetelaar, van den L.C.A.

1996-01-01

A recently developed spin coating method has been employed to produce a homogeneous distribution of nanometer-sized metal clusters onto a flat oxidic support. The particle size and distribution, and the total amount of material deposited has been studied by comparing the results of atomic force

Sapphire: a better material for atomization and in situ collection of silver volatile species for atomic absorption spectrometry

Energy Technology Data Exchange (ETDEWEB)

Musil, Stanislav, E-mail: stanomusil@biomed.cas.cz; Matoušek, Tomáš; Dědina, Jiří

2015-06-01

Sapphire is presented as a high temperature and corrosion resistant material of an optical tube of an atomizer for volatile species of Ag generated by the reaction with NaBH{sub 4}. The modular atomizer design was employed which allowed to carry out the measurements in two modes: (i) on-line atomization and (ii) in situ collection (directly in the optical tube) by means of excess of O{sub 2} over H{sub 2} in the carrier gas during the trapping step and vice versa in the volatilization step. In comparison with quartz atomizers, the sapphire tube atomizer provides a significantly increased atomizer lifetime as well as substantially improved repeatability of the Ag in situ collection signals shapes. In situ collection of Ag in the sapphire tube atomizer was highly efficient (> 90%). Limit of detection in the on-line atomization mode and in situ collection mode, respectively, was 1.2 ng ml{sup −1} and 0.15 ng ml{sup −1}. - Highlights: • Sapphire was tested as a new material of an atomizer tube for Ag volatile species. • Two measurement modes were investigated: on-line atomization and in situ collection. • In situ collection of Ag was highly efficient (> 90%) with LOD of 0.15 ng ml{sup −1}. • No devitrification of the sapphire tube observed in the course of several months.

Ground States of Ultracold Spin-1 Atoms in a Deep Double-Well Optical Superlattice in a Weak Magnetic Field

International Nuclear Information System (INIS)

Zheng Gong-Ping; Qin Shuai-Feng; Wang Shou-Yang; Jian Wen-Tian

2013-01-01

The ground states of the ultracold spin-1 atoms trapped in a deep one-dimensional double-well optical superlattice in a weak magnetic field are obtained. It is shown that the ground-state diagrams of the reduced double-well model are remarkably different for the antiferromagnetic and ferromagnetic condensates. The transition between the singlet state and nematic state is observed for the antiferromagnetic interaction atoms, which can be realized by modulating the tunneling parameter or the quadratic Zeeman energy. An experiment to distinguish the different spin states is suggested. (general)

Measuring the spin polarization of alkali-metal atoms using nuclear magnetic resonance frequency shifts of noble gases

Directory of Open Access Journals (Sweden)

X. H. Liu

2015-10-01

Full Text Available We report a novel method of measuring the spin polarization of alkali-metal atoms by detecting the NMR frequency shifts of noble gases. We calculated the profile of 87Rb D1 line absorption cross sections. We then measured the absorption profile of the sample cell, from which we calculated the 87Rb number densities at different temperatures. Then we measured the frequency shifts resulted from the spin polarization of the 87Rb atoms and calculated its polarization degrees at different temperatures. The behavior of frequency shifts versus temperature in experiment was consistent with theoretical calculation, which may be used as compensative signal for the NMRG closed-loop control system.

The spin polarized linear response from density functional theory: Theory and application to atoms

Energy Technology Data Exchange (ETDEWEB)

Fias, Stijn, E-mail: sfias@vub.ac.be; Boisdenghien, Zino; De Proft, Frank; Geerlings, Paul [General Chemistry (ALGC), Vrije Universiteit Brussel (Free University Brussels – VUB), Pleinlaan 2, 1050 Brussels (Belgium)

2014-11-14

Within the context of spin polarized conceptual density functional theory, the spin polarized linear response functions are introduced both in the [N, N{sub s}] and [N{sub α}, N{sub β}] representations. The mathematical relations between the spin polarized linear response functions in both representations are examined and an analytical expression for the spin polarized linear response functions in the [N{sub α}, N{sub β}] representation is derived. The spin polarized linear response functions were calculated for all atoms up to and including argon. To simplify the plotting of our results, we integrated χ(r, r′) to a quantity χ(r, r{sup ′}), circumventing the θ and ϕ dependence. This allows us to plot and to investigate the periodicity throughout the first three rows in the periodic table within the two different representations. For the first time, χ{sub αβ}(r, r{sup ′}), χ{sub βα}(r, r{sup ′}), and χ{sub SS}(r, r{sup ′}) plots have been calculated and discussed. By integration of the spin polarized linear response functions, different components to the polarisability, α{sub αα}, α{sub αβ}, α{sub βα}, and α{sub ββ} have been calculated.

Open quantum spin systems in semiconductor quantum dots and atoms in optical lattices

Energy Technology Data Exchange (ETDEWEB)

Schwager, Heike

2012-07-04

In this Thesis, we study open quantum spin systems from different perspectives. The first part is motivated by technological challenges of quantum computation. An important building block for quantum computation and quantum communication networks is an interface between material qubits for storage and data processing and travelling photonic qubits for communication. We propose the realisation of a quantum interface between a travelling-wave light field and the nuclear spins in a quantum dot strongly coupled to a cavity. Our scheme is robust against cavity decay as it uses the decay of the cavity to achieve the coupling between nuclear spins and the travelling-wave light fields. A prerequiste for such a quantum interface is a highly polarized ensemble of nuclear spins. High polarization of the nuclear spin ensemble is moreover highly desirable as it protects the potential electron spin qubit from decoherence. Here we present the theoretical description of an experiment in which highly asymmetric dynamic nuclear spin pumping is observed in a single self-assembled InGaAs quantum dot. The second part of this Thesis is devoted to fundamental studies of dissipative spin systems. We study general one-dimensional spin chains under dissipation and propose a scheme to realize a quantum spin system using ultracold atoms in an optical lattice in which both coherent interaction and dissipation can be engineered and controlled. This system enables the study of non-equilibrium and steady state physics of open and driven spin systems. We find, that the steady state expectation values of different spin models exhibit discontinuous behaviour at degeneracy points of the Hamiltonian in the limit of weak dissipation. This effect can be used to dissipatively probe the spectrum of the Hamiltonian. We moreover study spin models under the aspect of state preparation and show that dissipation drives certain spin models into highly entangled state. Finally, we study a spin chain with

Open quantum spin systems in semiconductor quantum dots and atoms in optical lattices

International Nuclear Information System (INIS)

Schwager, Heike

2012-01-01

In this Thesis, we study open quantum spin systems from different perspectives. The first part is motivated by technological challenges of quantum computation. An important building block for quantum computation and quantum communication networks is an interface between material qubits for storage and data processing and travelling photonic qubits for communication. We propose the realisation of a quantum interface between a travelling-wave light field and the nuclear spins in a quantum dot strongly coupled to a cavity. Our scheme is robust against cavity decay as it uses the decay of the cavity to achieve the coupling between nuclear spins and the travelling-wave light fields. A prerequiste for such a quantum interface is a highly polarized ensemble of nuclear spins. High polarization of the nuclear spin ensemble is moreover highly desirable as it protects the potential electron spin qubit from decoherence. Here we present the theoretical description of an experiment in which highly asymmetric dynamic nuclear spin pumping is observed in a single self-assembled InGaAs quantum dot. The second part of this Thesis is devoted to fundamental studies of dissipative spin systems. We study general one-dimensional spin chains under dissipation and propose a scheme to realize a quantum spin system using ultracold atoms in an optical lattice in which both coherent interaction and dissipation can be engineered and controlled. This system enables the study of non-equilibrium and steady state physics of open and driven spin systems. We find, that the steady state expectation values of different spin models exhibit discontinuous behaviour at degeneracy points of the Hamiltonian in the limit of weak dissipation. This effect can be used to dissipatively probe the spectrum of the Hamiltonian. We moreover study spin models under the aspect of state preparation and show that dissipation drives certain spin models into highly entangled state. Finally, we study a spin chain with

Non-collective oblate states in iodine isotopes at high spin

Energy Technology Data Exchange (ETDEWEB)

Paul, E S; Ali, I; Cullen, D M; Fallon, P; Forbes, S A; Hanna, F; Nolan, P J [Liverpool Univ. (United Kingdom). Oliver Lodge Lab.; Bentley, M A; Bruce, A M; Simpson, J [Daresbury Lab. (United Kingdom); Clark, R M; Regan, P H; Wadsworth, R [York Univ. (United Kingdom). Dept. of Physics; Fossan, D B; Hughes, J R; Lafosse, D R; Vaska, P; Waring, M P [Department of Physics, SUNY at Stony Brook, NY (United States); Liang, Y [Argonne National Lab., IL (United States); Ma, R [Brookhaven National Lab., Upton, NY (United States)

1992-08-01

Competition between single-particle and collective modes of excitation has been observed in the odd-A {sup 113-119}I isotopes at high spin. A maximally-aligned non-collective 43/2{sup -} configuration at {gamma}=+ 60 degrees is seen at similar excitation energies in these nuclei. 7 refs., 4 figs.

Atomic spin resonance in a rubidium beam obliquely incident to a transmission magnetic grating

International Nuclear Information System (INIS)

Hatakeyama, A; Goto, K

2016-01-01

We studied atomic spin resonance induced by atomic motion in a spatially periodic magnetostatic field. A rubidium atomic beam, with a velocity of about 400 m s −1 , was obliquely incident to a transmission magnetic grating that produced a spatially periodic magnetic field. The magnetic grating was formed by a magnetic thin film on a polyimide substrate that had multiple slits at 150 μm intervals. The atoms experienced field oscillation, depending on their velocity and the field period when passing through the grating, and underwent magnetic resonance. Resonance spectra obtained with a perpendicular magnetization film were in clear contrast to ones obtained with an in-plane magnetization film. The former exhibited resonance peaks at odd multiples of the frequency, determined by the velocity over the period, while the latter had dips at the same frequencies. (paper)

Simultaneous differential spinning disk fluorescence optical sectioning microscopy and nanomechanical mapping atomic force microscopy

International Nuclear Information System (INIS)

Miranda, Adelaide; De Beule, Pieter A. A.; Martins, Marco

2015-01-01

Combined microscopy techniques offer the life science research community a powerful tool to investigate complex biological systems and their interactions. Here, we present a new combined microscopy platform based on fluorescence optical sectioning microscopy through aperture correlation microscopy with a Differential Spinning Disk (DSD) and nanomechanical mapping with an Atomic Force Microscope (AFM). The illumination scheme of the DSD microscope unit, contrary to standard single or multi-point confocal microscopes, provides a time-independent illumination of the AFM cantilever. This enables a distortion-free simultaneous operation of fluorescence optical sectioning microscopy and atomic force microscopy with standard probes. In this context, we discuss sample heating due to AFM cantilever illumination with fluorescence excitation light. Integration of a DSD fluorescence optical sectioning unit with an AFM platform requires mitigation of mechanical noise transfer of the spinning disk. We identify and present two solutions to almost annul this noise in the AFM measurement process. The new combined microscopy platform is applied to the characterization of a DOPC/DOPS (4:1) lipid structures labelled with a lipophilic cationic indocarbocyanine dye deposited on a mica substrate

Simultaneous differential spinning disk fluorescence optical sectioning microscopy and nanomechanical mapping atomic force microscopy

Energy Technology Data Exchange (ETDEWEB)

Miranda, Adelaide; De Beule, Pieter A. A., E-mail: pieter.de-beule@inl.int [Applied Nano-Optics Laboratory, International Iberian Nanotechnology Laboratory, Avenida Mestre José Veiga, s/n, 4715-330 Braga (Portugal); Martins, Marco [Nano-ICs Group, International Iberian Nanotechnology Laboratory, Avenida Mestre José Veiga, s/n, 4715-330 Braga (Portugal)

2015-09-15

Combined microscopy techniques offer the life science research community a powerful tool to investigate complex biological systems and their interactions. Here, we present a new combined microscopy platform based on fluorescence optical sectioning microscopy through aperture correlation microscopy with a Differential Spinning Disk (DSD) and nanomechanical mapping with an Atomic Force Microscope (AFM). The illumination scheme of the DSD microscope unit, contrary to standard single or multi-point confocal microscopes, provides a time-independent illumination of the AFM cantilever. This enables a distortion-free simultaneous operation of fluorescence optical sectioning microscopy and atomic force microscopy with standard probes. In this context, we discuss sample heating due to AFM cantilever illumination with fluorescence excitation light. Integration of a DSD fluorescence optical sectioning unit with an AFM platform requires mitigation of mechanical noise transfer of the spinning disk. We identify and present two solutions to almost annul this noise in the AFM measurement process. The new combined microscopy platform is applied to the characterization of a DOPC/DOPS (4:1) lipid structures labelled with a lipophilic cationic indocarbocyanine dye deposited on a mica substrate.

Quasi-spin method in the case of j-j coupling in a shell of equivalent atomic electrons

International Nuclear Information System (INIS)

Savichyus, E.G.; Kanyauskas, Yu.M.; Rudzikas, Z.B.

1979-01-01

Mathematical apparatus of the theory of multielectronic atoms and ions in the case of j-j coupling in a shell of equivalent electrons is built. Quasi-spin method is used. The scheme of the investigation is the following: 1. Tensorial properties of the operators in quasi-spin space are considered. 2. Matrix elements of these operators are built and with the help of Wigner-Eckart theorem the dependence of the matrix elements upon the projection, including the quasi-spin projection, of the quantity of electrons in jj-subshell, is determined. 3. Subgenealogical coefficients (genealogical coefficients presented in quasi-spin space) are determined and some of their properties are investigated. The tables of subgenealogical coefficients for j=5/2, 7/2 are presented

Observation of the spin-orbit activated interchannel coupling in the 3d photoionization of caesium atoms

International Nuclear Information System (INIS)

Farrokhpour, H; Alagia, M; Amusia, M Ya

2006-01-01

The ionization cross-section of the 3d spin-orbit components of the Cs atom has been measured from about 12 to 70 eV above their respective thresholds. The measured relative ionization cross-section of the 3d 5/2 channel exhibits a pronounced minimum above threshold followed by a second maximum near the 3d 3/2 ionization onset and thus qualitatively confirms the theoretical predictions of a spin-orbit activated interchannel coupling (Amusia et al 2002 Phys. Rev. Lett 88 093002)

Observation of the spin-orbit activated interchannel coupling in the 3d photoionization of caesium atoms

Energy Technology Data Exchange (ETDEWEB)

Farrokhpour, H [Chemistry Department, Isfahan University of Technology, Isfahan 84154 (Iran, Islamic Republic of); Abdus Salam International Centre for Theoretical Physics, I-34014 Trieste (Italy); Alagia, M [CNR-ISMN Sez.Roma1, P.le A Moro 5, I-00185 Rome (Italy) and CNR-Lab. Naz. TASC-INFM, Gas Phase Beamline at Elettra, Area Science Park, I-34012 Basovizza, Trieste (Italy); Amusia, M Ya [Racah Institute of Physics, Hebrew University, Jerusalem 91904 (Israel); A F Ioffe Physical-Technical Institute, St Petersburg 194021 (Russian Federation)] (and others)

2006-02-21

The ionization cross-section of the 3d spin-orbit components of the Cs atom has been measured from about 12 to 70 eV above their respective thresholds. The measured relative ionization cross-section of the 3d{sub 5/2} channel exhibits a pronounced minimum above threshold followed by a second maximum near the 3d{sub 3/2} ionization onset and thus qualitatively confirms the theoretical predictions of a spin-orbit activated interchannel coupling (Amusia et al 2002 Phys. Rev. Lett 88 093002)

Hydride generation – in-atomizer collection of Pb in a quartz trap-and-atomizer device for atomic absorption spectrometry – an interference study

Energy Technology Data Exchange (ETDEWEB)

Novotný, Pavel [Institute of Analytical Chemistry of the ASCR, v.v.i., Veveří 97, 602 00 Brno (Czech Republic); High School in Hořice, Husova 1414, 508 01 Hořice (Czech Republic); Kratzer, Jan, E-mail: jkratzer@biomed.cas.cz [Institute of Analytical Chemistry of the ASCR, v.v.i., Veveří 97, 602 00 Brno (Czech Republic)

2013-01-01

Interferences of selected hydride forming elements (As, Sb, Bi, Se and Sn) on lead determination by hydride generation atomic absorption spectrometry were extensively studied in both on-line atomization and preconcentration (collection) modes. The commonly used on-line atomization mode was found free of significant interferences, whereas strong interference from Bi was observed when employing the preconcentration mode with plumbane collection in a quartz trap-and-atomizer device. Interference of Bi seems to take place in the preconcentration step. Interference of Bi in the collection mode cannot be reduced by increased hydrogen radical amount in the trap and/or the atomizer. - Highlights: ► Interference study on Pb determination by in-atomizer trapping was performed for the first time. ► Bi was found as a severe interferent in the preconcentration mode (Pb:Bi ratio 1:100). ► No interference was found in the on-line atomization (no preconcentration). ► Bi interference occurs during preconcentration.

Polarization-dependent pump-probe studies in atomic fine-structure levels: towards the production of spin-polarized electrons

International Nuclear Information System (INIS)

Sokell, E.; Zamith, S.; Bouchene, M.A.; Girard, B.

2000-01-01

The precession of orbital and spin angular momentum vectors has been observed in a pump-probe study of the 4P fine-structure states of atomic potassium. A femtosecond pump pulse prepared a coherent superposition of the two fine-structure components. A time-delayed probe pulse then ionized the system after it had been allowed to evolve freely. Oscillations recorded in the ion signal reflect the evolution of the orientation of the orbital and spin angular momentum due to spin-orbit coupling. This interpretation gives physical insight into the cause of the half-period phase shift observed when the relative polarizations of the laser pulses were changed from parallel to perpendicular. Finally, it is shown that these changes in the orientation of the spin momentum vector of the system can be utilized to produce highly spin-polarized free electrons on the femtosecond scale. (author)

Population of collective modes in light scattering by many atoms

Science.gov (United States)

Guerin, William; Kaiser, Robin

2017-05-01

The interaction of light with an atomic sample containing a large number of particles gives rise to many collective (or cooperative) effects, such as multiple scattering, superradiance, and subradiance, even if the atomic density is low and the incident optical intensity weak (linear optics regime). Tracing over the degrees of freedom of the light field, the system can be well described by an effective atomic Hamiltonian, which contains the light-mediated dipole-dipole interaction between atoms. This long-range interaction is at the origin of the various collective effects, or of collective excitation modes of the system. Even though an analysis of the eigenvalues and eigenfunctions of these collective modes does allow distinguishing superradiant modes, for instance, from other collective modes, this is not sufficient to understand the dynamics of a driven system, as not all collective modes are significantly populated. Here, we study how the excitation parameters, i.e., the driving field, determines the population of the collective modes. We investigate in particular the role of the laser detuning from the atomic transition, and demonstrate a simple relation between the detuning and the steady-state population of the modes. This relation allows understanding several properties of cooperative scattering, such as why superradiance and subradiance become independent of the detuning at large enough detuning without vanishing, and why superradiance, but not subradiance, is suppressed near resonance. We also show that the spatial properties of the collective modes allow distinguishing diffusive modes, responsible for radiation trapping, from subradiant modes.

Heralded entanglement of two remote atoms

Science.gov (United States)

Krug, Michael; Hofmann, Julian; Ortegel, Norbert; Gerard, Lea; Redeker, Kai; Henkel, Florian; Rosenfeld, Wenjamin; Weber, Markus; Weinfurter, Harald

2012-06-01

Entanglement between atomic quantum memories at remote locations will be a key resource for future applications in quantum communication. One possibility to generate such entanglement over large distances is entanglement swapping starting from two quantum memories each entangled with a photon. The photons can be transported to a Bell-state measurement where after the atomic quantum memories are projected onto an entangled state. We have set up two independently operated single atom experiments separated by 20 m. Via a spontaneous decay process each quantum memory, in our case a single Rb-87 atom, emits a single photon whose polarization is entangled with the atomic spin. The photons one emitted from each atom are collected into single-mode optical fibers guided to a non-polarizing 50-50 beam-splitter and detected by avalanche photodetectors. Bunching of indistinguishable photons allows to perform a Bell-state measurement on the photons. Conditioned on the registration of particular two-photon coincidences the spin states of both atoms are measured. The observed correlations clearly prove the entanglement of the two atoms. This is a first step towards creating a basic node of a quantum network as well as a key prerequisite for a future loophole-free test of Bell's inequality.

Dissipation-driven quantum phase transitions in collective spin systems

International Nuclear Information System (INIS)

Morrison, S; Parkins, A S

2008-01-01

We consider two different collective spin systems subjected to strong dissipation-on the same scale as interaction strengths and external fields-and show that either continuous or discontinuous dissipative quantum phase transitions can occur as the dissipation strength is varied. First, we consider a well-known model of cooperative resonance fluorescence that can exhibit a second-order quantum phase transition, and analyse the entanglement properties near the critical point. Next, we examine a dissipative version of the Lipkin-Meshkov-Glick interacting collective spin model, where we find that either first- or second-order quantum phase transitions can occur, depending only on the ratio of the interaction and external field parameters. We give detailed results and interpretation for the steady-state entanglement in the vicinity of the critical point, where it reaches a maximum. For the first-order transition we find that the semiclassical steady states exhibit a region of bistability. (fast track communication)

Ultracold Atoms in a Square Lattice with Spin-Orbit Coupling: Charge Order, Superfluidity, and Topological Signatures

Science.gov (United States)

Rosenberg, Peter; Shi, Hao; Zhang, Shiwei

2017-12-01

We present an ab initio, numerically exact study of attractive fermions in square lattices with Rashba spin-orbit coupling. The ground state of this system is a supersolid, with coexisting charge and superfluid order. The superfluid is composed of both singlet and triplet pairs induced by spin-orbit coupling. We perform large-scale calculations using the auxiliary-field quantum Monte Carlo method to provide the first full, quantitative description of the charge, spin, and pairing properties of the system. In addition to characterizing the exotic physics, our results will serve as essential high-accuracy benchmarks for the intense theoretical and especially experimental efforts in ultracold atoms to realize and understand an expanding variety of quantum Hall and topological superconductor systems.

Atom beams split by gentle persuasion

International Nuclear Information System (INIS)

Pool, R.

1994-01-01

Two different research teams have taken a big step toward atom interferometry. They have succeeded in splitting atomic beams by using atoms in spin states that neither absorb nor reemit laser light. By proper adjustment of experimental conditions, atoms are changed from one spin state to another, without passing through the intermediary excited state. The atoms in essence absorb momentum from the laser photons, without absorption or emission of photons. The change in momentum deflects atoms in the proper spin state

Monte Carlo simulations of phase transitions and lattice dynamics in an atom-phonon model for spin transition compounds

International Nuclear Information System (INIS)

Apetrei, Alin Marian; Enachescu, Cristian; Tanasa, Radu; Stoleriu, Laurentiu; Stancu, Alexandru

2010-01-01

We apply here the Monte Carlo Metropolis method to a known atom-phonon coupling model for 1D spin transition compounds (STC). These inorganic molecular systems can switch under thermal or optical excitation, between two states in thermodynamical competition, i.e. high spin (HS) and low spin (LS). In the model, the ST units (molecules) are linked by springs, whose elastic constants depend on the spin states of the neighboring atoms, and can only have three possible values. Several previous analytical papers considered a unique average value for the elastic constants (mean-field approximation) and obtained phase diagrams and thermal hysteresis loops. Recently, Monte Carlo simulation papers, taking into account all three values of the elastic constants, obtained thermal hysteresis loops, but no phase diagrams. Employing Monte Carlo simulation, in this work we obtain the phase diagram at T=0 K, which is fully consistent with earlier analytical work; however it is more complex. The main difference is the existence of two supplementary critical curves that mark a hysteresis zone in the phase diagram. This explains the pressure hysteresis curves at low temperature observed experimentally and predicts a 'chemical' hysteresis in STC at very low temperatures. The formation and the dynamics of the domains are also discussed.

Spin-polarized spin-orbit-split quantum-well states in a metal film

Energy Technology Data Exchange (ETDEWEB)

Varykhalov, Andrei; Sanchez-Barriga, Jaime; Gudat, Wolfgang; Eberhardt, Wolfgang; Rader, Oliver [BESSY Berlin (Germany); Shikin, Alexander M. [St. Petersburg State University (Russian Federation)

2008-07-01

Elements with high atomic number Z lead to a large spin-orbit coupling. Such materials can be used to create spin-polarized electronic states without the presence of a ferromagnet or an external magnetic field if the solid exhibits an inversion asymmetry. We create large spin-orbit splittings using a tungsten crystal as substrate and break the structural inversion symmetry through deposition of a gold quantum film. Using spin- and angle-resolved photoelectron spectroscopy, it is demonstrated that quantum-well states forming in the gold film are spin-orbit split and spin polarized up to a thickness of at least 10 atomic layers. This is a considerable progress as compared to the current literature which reports spin-orbit split states at metal surfaces which are either pure or covered by at most a monoatomic layer of adsorbates.

Nonequilibrium Spin Dynamics in a Trapped Fermi Gas with Effective Spin-Orbit Interactions

International Nuclear Information System (INIS)

Stanescu, Tudor D.; Zhang Chuanwei; Galitski, Victor

2007-01-01

We consider a trapped atomic system in the presence of spatially varying laser fields. The laser-atom interaction generates a pseudospin degree of freedom (referred to simply as spin) and leads to an effective spin-orbit coupling for the fermions in the trap. Reflections of the fermions from the trap boundaries provide a physical mechanism for effective momentum relaxation and nontrivial spin dynamics due to the emergent spin-orbit coupling. We explicitly consider evolution of an initially spin-polarized Fermi gas in a two-dimensional harmonic trap and derive nonequilibrium behavior of the spin polarization. It shows periodic echoes with a frequency equal to the harmonic trapping frequency. Perturbations, such as an asymmetry of the trap, lead to the suppression of the spin echo amplitudes. We discuss a possible experimental setup to observe spin dynamics and provide numerical estimates of relevant parameters

Anderson Transition of Cold Atoms with Synthetic Spin-Orbit Coupling in Two-Dimensional Speckle Potentials

Science.gov (United States)

Orso, Giuliano

2017-03-01

We investigate the metal-insulator transition occurring in two-dimensional (2D) systems of noninteracting atoms in the presence of artificial spin-orbit interactions and a spatially correlated disorder generated by laser speckles. Based on a high order discretization scheme, we calculate the precise position of the mobility edge and verify that the transition belongs to the symplectic universality class. We show that the mobility edge depends strongly on the mixing angle between Rashba and Dresselhaus spin-orbit couplings. For equal couplings a non-power-law divergence is found, signaling the crossing to the orthogonal class, where such a 2D transition is forbidden.

On the representation matrices of the spin permutation group. [for atomic and molecular electronic structures

Science.gov (United States)

Wilson, S.

1977-01-01

A method is presented for the determination of the representation matrices of the spin permutation group (symmetric group), a detailed knowledge of these matrices being required in the study of the electronic structure of atoms and molecules. The method is characterized by the use of two different coupling schemes. Unlike the Yamanouchi spin algebraic scheme, the method is not recursive. The matrices for the fundamental transpositions can be written down directly in one of the two bases. The method results in a computationally significant reduction in the number of matrix elements that have to be stored when compared with, say, the standard Young tableaux group theoretical approach.

Functionalizing carbon nitride with heavy atom-free spin converters for enhanced 1 O 2 generation

Energy Technology Data Exchange (ETDEWEB)

Wu, Wenting; Han, Congcong; Zhang, Qinhua; Zhang, Qinggang; Li, Zhongtao; Gosztola, David J.; Wiederrecht, Gary P.; Wu, Mingbo

2018-05-01

advanced photosensitizers for singlet oxygen (1O2) generation. However, the intersystem crossing (ISC) process is quite insufficient in carbon nitride, limiting the 1O2 generation. Here, we report a facile and general strategy to confined benzophenone as a heavy atom-free spin converter dopant in carbon nitride via the facile copolymerization. With proper energy level matching between the heavy atom-free spin converter and various ligands based on carbon nitride precursors, the proper combination can decrease the singlet-triplet energy gap (DEST) and hence generate 1O2 effectively. Due to its significant and selectivity for 1O2 generation, the as-prepared carbon nitride-based photosensitizer shows a high selective photooxidation activity for 1,5-dihydroxy-naphthalene (1,5-DHN). The product yield reached 71.8% after irradiation for 60 min, which was higher than that of cyclometalated PtII complexes (53.6%) in homogeneous photooxidation. This study can broaden the application of carbon nitride in the field of selective heterogeneous photooxidation due to simple operation, low cost, and high efficiency, making it a strong candidate for future industrialization.

Cooperative spin decoherence and population transfer

International Nuclear Information System (INIS)

Genes, C.; Berman, P. R.

2006-01-01

An ensemble of multilevel atoms is a good candidate for a quantum information storage device. The information is encrypted in the collective ground state atomic coherence, which, in the absence of external excitation, is decoupled from the vacuum and therefore decoherence free. However, in the process of manipulation of atoms with light pulses (writing, reading), one inadvertently introduces a coupling to the environment, i.e., a source of decoherence. The dissipation process is often treated as an independent process for each atom in the ensemble, an approach which fails at large atomic optical depths where cooperative effects must be taken into account. In this paper, the cooperative behavior of spin decoherence and population transfer for a system of two, driven multilevel atoms is studied. Not surprisingly, an enhancement in the decoherence rate is found, when the atoms are separated by a distance that is small compared to an optical wavelength; however, it is found that this rate increases even further for somewhat larger separations for atoms aligned along the direction of the driving field's propagation vector. A treatment of the cooperative modification of optical pumping rates and an effect of polarization swapping between atoms is also discussed, lending additional insight into the origin of the collective decay

Coherent Two-Dimensional Terahertz Magnetic Resonance Spectroscopy of Collective Spin Waves.

Science.gov (United States)

Lu, Jian; Li, Xian; Hwang, Harold Y; Ofori-Okai, Benjamin K; Kurihara, Takayuki; Suemoto, Tohru; Nelson, Keith A

2017-05-19

We report a demonstration of two-dimensional (2D) terahertz (THz) magnetic resonance spectroscopy using the magnetic fields of two time-delayed THz pulses. We apply the methodology to directly reveal the nonlinear responses of collective spin waves (magnons) in a canted antiferromagnetic crystal. The 2D THz spectra show all of the third-order nonlinear magnon signals including magnon spin echoes, and 2-quantum signals that reveal pairwise correlations between magnons at the Brillouin zone center. We also observe second-order nonlinear magnon signals showing resonance-enhanced second-harmonic and difference-frequency generation. Numerical simulations of the spin dynamics reproduce all of the spectral features in excellent agreement with the experimental 2D THz spectra.

Theory of Collective Spin-Wave Modes of Interacting Ferromagnetic Spheres

Science.gov (United States)

2004-09-29

Office (Durham) through Contract No. CS0001028. R. A. thanks also Proyecto Fondecyt Grant No. 7030063. *Present address: Universidad de Chile...Departamento de Fisica FCFM, Santiago, Chile. 1 For examples of experimental studies of the collective spin wave modes of superlattices and multilayers, see M...character to those shown above. In this case, there is no simple symmetry de - composition one canmake for the collective modes, so all branches appear

Quantum simulation of spin models on an arbitrary lattice with trapped ions

International Nuclear Information System (INIS)

Korenblit, S; Kafri, D; Campbell, W C; Islam, R; Edwards, E E; Monroe, C; Gong, Z-X; Lin, G-D; Duan, L-M; Kim, J; Kim, K

2012-01-01

A collection of trapped atomic ions represents one of the most attractive platforms for the quantum simulation of interacting spin networks and quantum magnetism. Spin-dependent optical dipole forces applied to an ion crystal create long-range effective spin–spin interactions and allow the simulation of spin Hamiltonians that possess nontrivial phases and dynamics. Here we show how the appropriate design of laser fields can provide for arbitrary multidimensional spin–spin interaction graphs even for the case of a linear spatial array of ions. This scheme uses currently available trap technology and is scalable to levels where the classical methods of simulation are intractable. (paper)

Collective vs atomic models of the hadrons

International Nuclear Information System (INIS)

Stokar, S.

1983-02-01

We examine the relationship between heavy and light quark systems. Using a Bogoliubov-Valatin transformation we show how to interpolate continuously between heavy quark atomic models and light quark collective models of the hadrons. (author)

Measurement-Based Entanglement of Noninteracting Bosonic Atoms.

Science.gov (United States)

Lester, Brian J; Lin, Yiheng; Brown, Mark O; Kaufman, Adam M; Ball, Randall J; Knill, Emanuel; Rey, Ana M; Regal, Cindy A

2018-05-11

We demonstrate the ability to extract a spin-entangled state of two neutral atoms via postselection based on a measurement of their spatial configuration. Typically, entangled states of neutral atoms are engineered via atom-atom interactions. In contrast, in our Letter, we use Hong-Ou-Mandel interference to postselect a spin-singlet state after overlapping two atoms in distinct spin states on an effective beam splitter. We verify the presence of entanglement and determine a bound on the postselected fidelity of a spin-singlet state of (0.62±0.03). The experiment has direct analogy to creating polarization entanglement with single photons and hence demonstrates the potential to use protocols developed for photons to create complex quantum states with noninteracting atoms.

Comparison of interacting boson-fermion model with spin-dependent generalized collective model for the j=3/2

International Nuclear Information System (INIS)

Baktybaev, K.; Koilyk, N.; Ramankulov, K.

2006-01-01

Full text: Collective Schrodinger equations are applied to describe low-energy spectra of even-even nuclei [1]. Spectra for even-odd nuclei are calculated by coupling the single particle degrees of freedom to the collective degree of freedom of the core nucleus, which is of even-even type. The collective spin has a value of 3/2. This leads to the assumption that the linearized equation may be applied to describe nuclei with spin 3/2 in the ground state. Good description of the low energy spectra and electromagnetic transition probabilities can be obtained only with introduction of spin-dependent potentials, which apart from coordinates and momenta also depend on the matrices of the Clifford algebra arising in the linearization,. The interacting boson-fermion models (IBFM) [2] represent another approach to describe spectra of even-odd nuclei. For even-odd nuclei with spin 3/2 in the ground state one uses so-called j=3/2 - IBFM, which is also denoted as the U B (6)xU F (4) IBFM. In this paper we establish the relation between the matrices of the Clifford algebra, which arise in the linearization procedure, and the fermion operators of the j=3/2 IBFM. This allows us to establish a connection between the j=3/2 IBFM and spin dependent generalized collective model (SGCM). The results of the SGCM for Ir and Au nuclei are presented and compared with the results of the j=3/2 IBFM with a dynamical spin symmetry [3] present. In this respect we could apply the linearized collective Schrodinger equation and IBFM with arbitrary spin to all other even-odd nuclei. (author)

High-Frequency Dynamics Modulated by Collective Magnetization Reversal in Artificial Spin Ice

Energy Technology Data Exchange (ETDEWEB)

Jungfleisch, Matthias B.; Sklenar, Joseph; Ding, Junjia; Park, Jungsik; Pearson, John E.; Novosad, Valentine; Schiffer, Peter; Hoffmann, Axel

2017-12-01

Spin-torque ferromagnetic resonance arises in heavy metal-ferromagnet heterostructures when an alternating charge current is passed through the bilayer stack. The methodology to detect the resonance is based on the anisotropic magnetoresistance, which is the change in the electrical resistance due to different orientations of the magnetization. In connected networks of ferromagnetic nanowires, known as artificial spin ice, the magnetoresistance is rather complex owing to the underlying collective behavior of the geometrically frustrated magnetic domain structure. Here, we demonstrate spin-torque ferromagnetic resonance investigations in a square artificial spin-ice system and correlate our observations to magneto-transport measurements. The experimental findings are described using a simulation approach that highlights the importance of the correlated dynamics response of the magnetic system. Our results open the possibility of designing reconfigurable microwave oscillators and magnetoresistive devices based on connected networks of nanomagnets.

High-Frequency Dynamics Modulated by Collective Magnetization Reversal in Artificial Spin Ice

Science.gov (United States)

Jungfleisch, Matthias B.; Sklenar, Joseph; Ding, Junjia; Park, Jungsik; Pearson, John E.; Novosad, Valentine; Schiffer, Peter; Hoffmann, Axel

2017-12-01

Spin-torque ferromagnetic resonance arises in heavy metal-ferromagnet heterostructures when an alternating charge current is passed through the bilayer stack. The methodology to detect the resonance is based on the anisotropic magnetoresistance, which is the change in the electrical resistance due to different orientations of the magnetization. In connected networks of ferromagnetic nanowires, known as artificial spin ice, the magnetoresistance is rather complex owing to the underlying collective behavior of the geometrically frustrated magnetic domain structure. Here, we demonstrate spin-torque ferromagnetic resonance investigations in a square artificial spin-ice system and correlate our observations to magnetotransport measurements. The experimental findings are described using a simulation approach that highlights the importance of the correlated dynamics response of the magnetic system. Our results open the possibility of designing reconfigurable microwave oscillators and magnetoresistive devices based on connected networks of nanomagnets.

Squeezing of Collective Excitations in Spin Ensembles

DEFF Research Database (Denmark)

Kraglund Andersen, Christian; Mølmer, Klaus

2012-01-01

We analyse the possibility to create two-mode spin squeezed states of two separate spin ensembles by inverting the spins in one ensemble and allowing spin exchange between the ensembles via a near resonant cavity field. We investigate the dynamics of the system using a combination of numerical an...

Photoionization of Endohedral Atoms: Collective, Reflective and Collateral Emissions

International Nuclear Information System (INIS)

Chakraborty, Himadri S.; McCune, Matthew A.; Hopper, Dale E.; Madjet, Mohamed E.; Manson, Steven T.

2009-01-01

The photoionization properties of a fullerene-confined atom differ dramatically from that of an isolated atom. In the low energy region, where the fullerene plasmons are active, the electrons of the confined atom emerge through a collective channel carrying a significant chunk of plasmon with it. The photoelectron angular distribution of the confined atom however shows far lesser impact of the effect. At higher energies, the interference between two single-electron ionization channels, one directly from the atom and another reflected off the fullerene cage, producuces oscillatory cross sections. But for the outermost atomic level, which transfers some electrons to the cage, oscillations are further modulated by the collateral emission from the part of the atomic charge density transferred to the cage. These various modes of emissions are studied for the photoionization of Ar endohedrally confined in C 60 .

Hong-Ou-Mandel Interference between Two Deterministic Collective Excitations in an Atomic Ensemble

Science.gov (United States)

Li, Jun; Zhou, Ming-Ti; Jing, Bo; Wang, Xu-Jie; Yang, Sheng-Jun; Jiang, Xiao; Mølmer, Klaus; Bao, Xiao-Hui; Pan, Jian-Wei

2016-10-01

We demonstrate deterministic generation of two distinct collective excitations in one atomic ensemble, and we realize the Hong-Ou-Mandel interference between them. Using Rydberg blockade we create single collective excitations in two different Zeeman levels, and we use stimulated Raman transitions to perform a beam-splitter operation between the excited atomic modes. By converting the atomic excitations into photons, the two-excitation interference is measured by photon coincidence detection with a visibility of 0.89(6). The Hong-Ou-Mandel interference witnesses an entangled NOON state of the collective atomic excitations, and we demonstrate its two times enhanced sensitivity to a magnetic field compared with a single excitation. Our work implements a minimal instance of boson sampling and paves the way for further multimode and multiexcitation studies with collective excitations of atomic ensembles.

Theory of single-spin inelastic tunneling spectroscopy.

Science.gov (United States)

Fernández-Rossier, J

2009-06-26

I show that recent experiments of inelastic scanning tunneling spectroscopy of single and a few magnetic atoms are modeled with a phenomenological spin-assisted tunneling Hamiltonian so that the inelastic dI/dV line shape is related to the spin spectral weight of the magnetic atom. This accounts for the spin selection rules and dI/dV spectra observed experimentally for single Fe and Mn atoms deposited on Cu2N. In the case of chains of Mn atoms it is found necessary to include both first and second-neighbor exchange interactions as well as single-ion anisotropy.

Inhomogeneous Spin Diffusion in Traps with Cold Atoms

DEFF Research Database (Denmark)

Heiselberg, Henning

2012-01-01

increases. The inhomogeneity and the smaller nite trap size signicantly reduce the spin diusion rate at low temperatures. The resulting spin diusion rates and spin drag at longer time scales are compatible with measurements at low to high temperatures for resonant attractive interactions...

Spin alignment and collective moment of inertia of the basic rotational band in the cranking model

International Nuclear Information System (INIS)

Tanaka, Yoshihide

1982-01-01

By making an attempt to separate the intrinsic particle and collective rotational motions in the cranking model, the spin alignment and the collective moment of inertia characterizing the basic rotational bands are defined, and are investigated by using a simple i sub(13/2) shell model. The result of the calculation indicates that the collective moment of inertia decreases under the presence of the quasiparticles which are responsible for the increase of the spin alignment of the band. (author)

Enhanced spin polarization of elastic electron scattering from alkaline-earth-metal atoms in Ramsauer-Townsend and low-lying shape resonance regions

International Nuclear Information System (INIS)

Yuan, J.; Zhang, Z.

1993-01-01

Spin polarizations (SP's) of elastic electron scattering from alkaline-earth-metal atoms in Ramsauer-Townsend (RT) and low-lying shape resonance (SR) regions are calculated using a relativistic method. The detailed SP distributions both with scattering angle and with electron energy are presented via the energy- and angle-dependent surfaces of SP parameters. It is shown that the SP effects of the collisions of electrons with Ca, Sr, and Ba atoms in the RT region are significant in a considerable area on the energy-angle plane and that the spin-orbit interaction is well increased around the low-lying p-wave SR states of Be and Mg and the d-wave SR states of Ca, Sr, and Ba

Low energy collisions of spin-polarized metastable argon atoms with ground state argon atoms

Science.gov (United States)

Taillandier-Loize, T.; Perales, F.; Baudon, J.; Hamamda, M.; Bocvarski, V.; Ducloy, M.; Correia, F.; Fabre, N.; Dutier, G.

2018-04-01

The collision between a spin-polarized metastable argon atom in Ar* (3p54s, 3P2, M = +2) state slightly decelerated by the Zeeman slower-laser technique and a co-propagating thermal ground state argon atom Ar (3p6, 1S0), both merged from the same supersonic beam, but coming through adjacent slots of a rotating disk, is investigated at the center of mass energies ranging from 1 to 10 meV. The duration of the laser pulse synchronised with the disk allows the tuning of the relative velocity and thus the collision energy. At these sub-thermal energies, the ‘resonant metastability transfer’ signal is too small to be evidenced. The explored energy range requires using indiscernibility amplitudes for identical isotopes to have a correct interpretation of the experimental results. Nevertheless, excitation transfers are expected to increase significantly at much lower energies as suggested by previous theoretical predictions of potentials 2g(3P2) and 2u(3P2). Limits at ultra-low collisional energies of the order of 1 mK (0.086 μeV) or less, where gigantic elastic cross sections are expected, will also be discussed. The experimental method is versatile and could be applied using different isotopes of Argon like 36Ar combined with 40Ar, as well as other rare gases among which Krypton should be of great interest thanks to the available numerous isotopes present in a natural gas mixture.

Electron spin resonance of the solvation of radiation-produced silver atoms in alcohol-water mixtures

International Nuclear Information System (INIS)

Li, A.S.W.; Kevan, L.

1982-01-01

Frozen solutions of silver salts exposed to 60 Co γ-irradiation form silver atoms by reaction of radiation-produced electrons with the silver ion. At 4 K the silver atoms are initially produced in a nonequilibrium or presolvated state and upon brief thermal excitation to 77 K the first solvation shell geometry changes towards an equilibrium or solvated silver atom. This is most pronounced in water but also occurs in methanol, ethanol and n-propanol matrices. The changes in the electron spin resonance magnetic parameters upon silver atom solvation have been determined. In alcohol-water mixtures Ag 0 is preferentially solvated by polycrystalline water at low alcohol concentration. Above a particular alcohol mole percent Ag 0 suddenly changes its environment to a glassy alcohol one. This sudden change occurs at 17, 13 and 6 mol % methanol, ethanol and n-propanol, respectively. These mole percents correlate with the minimum of the excess enthalpy of mixing and with the hydrogen atom trapping ability of these alcohol-water mixtures. The results also suggest that the local environmental disorder around Ag 0 increases with alcohol chain length in alcohol-water frozen solutions. (author)

A novel Cs-(129)Xe atomic spin gyroscope with closed-loop Faraday modulation.

Science.gov (United States)

Fang, Jiancheng; Wan, Shuangai; Qin, Jie; Zhang, Chen; Quan, Wei; Yuan, Heng; Dong, Haifeng

2013-08-01

We report a novel Cs-(129)Xe atomic spin gyroscope (ASG) with closed-loop Faraday modulation method. This ASG requires approximately 30 min to start-up and 110 °C to operate. A closed-loop Faraday modulation method for measurement of the optical rotation was used in this ASG. This method uses an additional Faraday modulator to suppress the laser intensity fluctuation and Faraday modulator thermal induced fluctuation. We theoretically and experimentally validate this method in the Cs-(129)Xe ASG and achieved a bias stability of approximately 3.25 °∕h.

Bandwidth broadening and asymmetric softening of collective spin waves in magnonic crystals

International Nuclear Information System (INIS)

Montoncello, F.; Giovannini, L.

2014-01-01

We investigate the dependence on the applied field of the frequency/wavevector dispersion relations of collective spin waves in arrays of dots, close to a magnetic transition. In particular, we focus on the low frequency “soft” modes in three different cases: end modes in the transition between two different saturated states in ellipses, fundamental mode in the saturated-to-vortex transition in disks, and gyrotropic mode in the vortex-to-saturated transition in disks. Noteworthy, the spin waves with nonzero Bloch wavevector along the direction of the applied field happen to soften earlier than spin waves with a Bloch wavevector along different directions, and this feature is responsible for an asymmetric broadening of the bandwidth along the different lattice directions. This is particularly useful in magnonic/spin-logic device research, if different binary digits are associated to modes with the same cell function but different propagation directions.

Sub-Shot-Noise Magnetometry with a Correlated Spin-Relaxation Dominated Alkali-Metal Vapor

International Nuclear Information System (INIS)

Kominis, I. K.

2008-01-01

Spin noise sets fundamental limits to the precision of measurements using spin-polarized atomic vapors, such as performed with sensitive atomic magnetometers. Spin squeezing offers the possibility to extend the measurement precision beyond the standard quantum limit of uncorrelated atoms. Contrary to current understanding, we show that, even in the presence of spin relaxation, spin squeezing can lead to a significant reduction of spin noise, and hence an increase in magnetometric sensitivity, for a long measurement time. This is the case when correlated spin relaxation due to binary alkali-atom collisions dominates independently acting decoherence processes, a situation realized in thermal high atom-density magnetometers and clocks

Atomic structures of the rare-earths and actinides via relativistic current- and spin-density functional theory

International Nuclear Information System (INIS)

Higuchi, M.; Onuki, Y.; Osaka Univ., Toyonaka; Hasegawa, A.

1998-01-01

A new single-particle equation of the Kohn-Sham-Dirac type is derived from a relativistic current- and spin-density functional theory (RCSDFT), and is here applied to the calculations of the atomic structures of the rare-earth elements. Both the relativistic effects and the magnetic effects are taken into account on an equal footing, and the numerical calculation is carried out by modifying the method of Cortona et al. Because of the presence of the effective magnetic field, the degeneracies in all orbits are completely resolved like the Zeeman splittings. Total spin and orbital angular momenta over all the occupied states are shown to agree reasonably well with the Hund's rules for the rare-earth ions. (orig.)

Quantum and semiclassical spin networks: from atomic and molecular physics to quantum computing and gravity

Science.gov (United States)

Aquilanti, Vincenzo; Bitencourt, Ana Carla P.; Ferreira, Cristiane da S.; Marzuoli, Annalisa; Ragni, Mirco

2008-11-01

The mathematical apparatus of quantum-mechanical angular momentum (re)coupling, developed originally to describe spectroscopic phenomena in atomic, molecular, optical and nuclear physics, is embedded in modern algebraic settings which emphasize the underlying combinatorial aspects. SU(2) recoupling theory, involving Wigner's 3nj symbols, as well as the related problems of their calculations, general properties, asymptotic limits for large entries, nowadays plays a prominent role also in quantum gravity and quantum computing applications. We refer to the ingredients of this theory—and of its extension to other Lie and quantum groups—by using the collective term of 'spin networks'. Recent progress is recorded about the already established connections with the mathematical theory of discrete orthogonal polynomials (the so-called Askey scheme), providing powerful tools based on asymptotic expansions, which correspond on the physical side to various levels of semi-classical limits. These results are useful not only in theoretical molecular physics but also in motivating algorithms for the computationally demanding problems of molecular dynamics and chemical reaction theory, where large angular momenta are typically involved. As for quantum chemistry, applications of these techniques include selection and classification of complete orthogonal basis sets in atomic and molecular problems, either in configuration space (Sturmian orbitals) or in momentum space. In this paper, we list and discuss some aspects of these developments—such as for instance the hyperquantization algorithm—as well as a few applications to quantum gravity and topology, thus providing evidence of a unifying background structure.

A collection of formulas for spin dependent deep inelastic scattering

International Nuclear Information System (INIS)

Pussieux, T.

1995-03-01

The analysis of the longitudinal spin structure functions of the proton, neutron and deuteron requires the use of a large number of formulas and numerical inputs taken from various unpolarized experiments. The aim of this report is to collect this information which is usually scattered in the literature. (author). 26 refs., 3 figs., 1 tab

Spin Drag and Spin-Charge Separation in Cold Fermi Gases

International Nuclear Information System (INIS)

Polini, Marco; Vignale, Giovanni

2007-01-01

Low-energy spin and charge excitations of one-dimensional interacting fermions are completely decoupled and propagate with different velocities. These modes, however, can decay due to several possible mechanisms. In this Letter we expose a new facet of spin-charge separation: not only the speeds but also the damping rates of spin and charge excitations are different. While the propagation of long-wavelength charge excitations is essentially ballistic, spin propagation is intrinsically damped and diffusive. We suggest that cold Fermi gases trapped inside a tight atomic waveguide offer the opportunity to measure the spin-drag relaxation rate that controls the broadening of a spin packet

Measurement of complete and continuous Wigner functions for discrete atomic systems

Science.gov (United States)

Tian, Yali; Wang, Zhihui; Zhang, Pengfei; Li, Gang; Li, Jie; Zhang, Tiancai

2018-01-01

We measure complete and continuous Wigner functions of a two-level cesium atom in both a nearly pure state and highly mixed states. We apply the method [T. Tilma et al., Phys. Rev. Lett. 117, 180401 (2016), 10.1103/PhysRevLett.117.180401] of strictly constructing continuous Wigner functions for qubit or spin systems. We find that the Wigner function of all pure states of a qubit has negative regions and the negativity completely vanishes when the purity of an arbitrary mixed state is less than 2/3 . We experimentally demonstrate these findings using a single cesium atom confined in an optical dipole trap, which undergoes a nearly pure dephasing process. Our method can be applied straightforwardly to multi-atom systems for measuring the Wigner function of their collective spin state.

Correlations between atomic structure and giant magnetoresistance ratio in Co2(Fe,Mn)Si spin valves

International Nuclear Information System (INIS)

Lari, L; Sizeland, J; Gilks, D; Uddin, G M; Nedelkoski, Z; Hasnip, P J; Lazarov, V K; Yoshida, K; Galindo, P L; Sato, J; Oogane, M; Ando, Y; Hirohata, A

2014-01-01

We show that the magnetoresistance of Co 2 Fe x Mn 1−x Si-based spin valves, over 70% at low temperature, is directly related to the structural ordering in the electrodes and at the electrodes/spacer (Co 2 Fe x Mn 1−x Si/Ag) interfaces. Aberration-corrected atomic resolution Z-contrast scanning transmission electron microscopy of device structures reveals that annealing at 350 °C and 500 °C creates partial B2/L2 1 and fully L2 1 ordering of electrodes, respectively. Interface structural studies show that the Ag/Co 2 Fe x Mn 1−x Si interface is more ordered compared to the Co 2 Fe x Mn 1−x Si/Ag interface. The release of interface strain is mediated by misfit dislocations that localize the strain around the dislocation cores, and the effect of this strain is assessed by first principles electronic structure calculations. This study suggests that by improving the atomic ordering and strain at the interfaces, further enhancement of the magnetoresistance of CFMS-based current-perpendicular-to-plane spin valves is possible. (fast track communication)

Collective properties and shapes of nuclei at very high spins

International Nuclear Information System (INIS)

Johnson, N.R.

1991-01-01

A topic which has been of major interest to us for some years now involves the evolution of nuclear collectivity at high rotational frequencies and the accompanying changes in the shapes of nuclei in these extreme conditions. We carry out these studies by determining the dynamic electromagnetic multipole moments which are a reflection of the collective aspects of the nuclear wave functions. The most direct way to get these multipole moments is by measurements of excited-state lifetimes which provide the transition matrix elements in a fairly straightforward fashion. Although the primary emphasis of this paper is on the collectivity of the high-spin states in 160 Yb and 164 Yb, it is important to review briefly some work we began about ten years ago lifetime studies of moderately high spins in nuclei near N=90 using the recoil-distance (RD) method. These nuclei are just at the onset of permanent deformation and are known to be very soft with respect to deformation changes. This softness is clearly illustrated in contour diagrams of their potential-energy surfaces. For example, the potential energy surface of 160 Yb reveals that the minimum in the potential occurs around var-epsilon ∼ 0.2 and that it is very shallow in the γ degree of freedom. Because of their γ softness, we have studied several nuclei near N=90 to assess to what extent the polarization effects induced by rotation alignment of high-j quasiparticles affect their collectivity

Nuclear spin polarization of targets

International Nuclear Information System (INIS)

Happer, W.

1990-01-01

Lasers can be used to produce milligrams to grams of noble gas nuclei with spin polarizations in excess of 50%. These quantities are sufficient to be very useful targets in nuclear physics experiments. Alkali-metal atoms are used to capture the angular momentum of circularly polarized laser photons, and the alkali-metal atoms transfer their angular momentum to noble gas atoms in binary or three-body collisions. Non-radiative collisions between the excited alkali atoms and molecular quenching gases are essential to avoid radiation trapping. The spin exchange can involve gas-phase van der Waals molecules, consisting of a noble gas atom and an alkali metal atom. Surface chemistry is also of great importance in determining the wall-induced relaxation rates of the noble gases

Collective excitations in circular atomic configurations and single-photon traps

International Nuclear Information System (INIS)

Hammer, Hanno

2004-01-01

Correlated excitations in a plane circular configuration of identical atoms with parallel dipole moments are investigated. The collective energy eigenstates, which are formally identical to Frenkel excitons, can be computed together with their level shifts and decay rates by decomposing the atomic state space into carrier spaces for the irreducible representations of the symmetry group Z N of the circle. It is shown that the index p of these representations can be used as a quantum number analogously to the orbital angular momentum quantum number l in hydrogenlike systems. Just as the hydrogen s states are the only electronic wave functions which can occupy the central region of the Coulomb potential, the quasiparticle corresponding to a collective excitation of the atoms in the circle can occupy the central atom only for vanishing Z N quantum number p. If a central atom is present, the p=0 state splits into two and shows level crossing at certain radii; in the regions between these radii, damped quantum beats between two 'extreme' p=0 configurations occur. The physical mechanisms behind super- and subradiance at a given radius are discussed. It is shown that, beyond a certain critical number of atoms in the circle, the lifetime of the maximally subradiant state increases exponentially with the number of atoms in the configuration, making the system a natural candidate for a single-photon trap

Electronic readout of a single nuclear spin using a molecular spin transistor

Science.gov (United States)

Vincent, R.; Klyastskaya, S.; Ruben, M.; Wernsdorfer, W.; Balestro, F.

2012-02-01

Quantum control of individual spins in condensed matter devices is an emerging field with a wide range of applications ranging from nanospintronics to quantum computing [1,2]. The electron, with its spin and orbital degrees of freedom, is conventionally used as carrier of the quantum information in the devices proposed so far. However, electrons exhibit a strong coupling to the environment leading to reduced relaxation and coherence times. Indeed quantum coherence and stable entanglement of electron spins are extremely difficult to achieve. We propose a new approach using the nuclear spin of an individual metal atom embedded in a single-molecule magnet (SMM). In order to perform the readout of the nuclear spin, the quantum tunneling of the magnetization (QTM) of the magnetic moment of the SMM in a transitor-like set-up is electronically detected. Long spin lifetimes of an individual nuclear spin were observed and the relaxation characteristics were studied. The manipulation of the nuclear spin state of individual atoms embedded in magnetic molecules opens a completely new world, where quantum logic may be integrated.[4pt] [1] L. Bogani, W. Wernsdorfer, Nature Mat. 7, 179 (2008).[0pt] [2] M. Urdampilleta, S. Klyatskaya, J.P. Cleuziou, M. Ruben, W. Wernsdorfer, Nature Mat. 10, 502 (2011).

Collective effects in isolated atoms (many-body aspects of photoionization process)

International Nuclear Information System (INIS)

Amusia, M.Y.

1983-01-01

This chapter examines outer and intermediate many-electron shells and demonstrates that photoionization is of collective nature because in the atomic reaction to the external electromagnetic field at least all electrons of the ionized subshell take part. Performs the calculation of complex atom photoionization using random phase approximation with exchange (RPAE). Explains that in RPAE the ionization amplitude is presented as a sum of two terms, describing the direct knock-out and the induced one which is connected with a variation of the self-consistent field, caused by polarization of atomic shells under the action of the external field. Discusses collective effects in outer shells; deviation from RPAE prediction in outer shells; excitations ''two electrons-two holes'' and autoionizing states; collective effects in inner shells; and bremsstrahlung. Observes a large number of many-particle effects which manifest themselves practically in all atomic processes. Finds that by correcting and improving the one-electron approximation it becomes possible even in its frame to include much of what seems to be many-electron corrections

Spin-selective depopulation of triplet sublevels in rapidly rotating triplet exciplexes detected by a heavy-atom-induced magnetic field effect

OpenAIRE

Steiner, Ulrich

1980-01-01

A mechanism is presented explaining a reported heavy-atom-induced magnetic field effect as a consequence of non-equilibrium triplet sublevel population in an intermediate exciplex. The triplet exciplex spin polarization is induced by sub-level-selective intersystem crossing from the exciplex triplet to its singlet ground state and is decreased by an external magnetic field. The theory accounts almost quantitatively for the observed influence of magnetic field strength and heavy-atom substitue...

Relativistic electron-atom scattering in an extremely powerful laser field: Relevance of spin effects

International Nuclear Information System (INIS)

Panek, P.; Kaminski, J.Z.; Ehlotzky, F.

2002-01-01

We reconsider the relativistic scattering of electrons by an atom, being approximated by a static potential, in an extremely powerful electromagnetic plane wave of frequency ω and linear polarization ε. Since to a first order of approximation spin effects can be neglected, we first describe the scattered electron by the Gordon solution of the Klein-Gordon equation. Then we investigate the same scattering process by including the spin effects, using for the electron the Volkov solution of the Dirac equation. For sufficiently energetic electrons, the first-order Born approximation can be employed to represent the corresponding scattering matrix element. We compare the results of the differential cross sections of induced and inverse bremsstrahlung, evaluated from both approximations, for various parameter values and angular configurations and we find that in most cases the spin effects are marginal, even at very high laser power. On the other hand, we recover the various asymmetries in the angular distributions of the scattered electrons and their respective energies due to the laser-induced drift motion of the electrons in the direction of propagation of the radiation field, thus confirming the findings of our previous work [Phys. Rev. A 59, 2105 (1999); Laser Physics 10, 163 (2000)

Role of atomic spin-mechanical coupling in the problem of a magnetic biocompass

Science.gov (United States)

Cao, Yunshan; Yan, Peng

2018-04-01

It is a well established notion that animals can detect the Earth's magnetic field, while the biophysical origin of such magnetoreception is still elusive. Recently, a magnetic receptor Drosophila CG8198 (MagR) with a rodlike protein complex is reported [S. Qin et al., Nat. Mater. 15, 217 (2016), 10.1038/nmat4484] to act like a compass needle to guide the magnetic orientation of animals. This view, however, is challenged [M. Meister, Elife 5, e17210 (2016), 10.7554/eLife.17210] by arguing that thermal fluctuations beat the Zeeman coupling of the proteins's magnetic moment with the rather weak geomagnetic field (˜25 -65 μ T ). In this work, we show that the spin-mechanical interaction at the atomic scale gives rise to a high blocking temperature which allows a good alignment of the protein's magnetic moment with the Earth's magnetic field at room temperature. Our results provide a promising route to resolve the debate on the thermal behaviors of MagR, and may stimulate a broad interest in spin-mechanical couplings down to atomistic levels.

Towards spin injection into silicon

Energy Technology Data Exchange (ETDEWEB)

Dash, S.P.

2007-08-15

Si has been studied for the purpose of spin injection extensively in this thesis. Three different concepts for spin injection into Si have been addressed: (1) spin injection through a ferromagnet-Si Schottky contact, (2) spin injection using MgO tunnel barriers in between the ferromagnet and Si, and (3) spin injection from Mn-doped Si (DMS) as spin aligner. (1) FM-Si Schottky contact for spin injection: To be able to improve the interface qualities one needs to understand the atomic processes involved in the formation of silicide phases. In order to obtain more detailed insight into the formation of such phases the initial stages of growth of Co and Fe were studied in situ by HRBS with monolayer depth resolution.(2) MgO tunnel barrier for spin injection into Si: The fabrication and characterization of ultra-thin crystalline MgO tunnel barriers on Si (100) was presented. (3) Mn doped Si for spin injection: Si-based diluted magnetic semiconductor samples were prepared by doping Si with Mn by two different methods i) by Mn ion implantation and ii) by in-diffusion of Mn atoms (solid state growth). (orig.)

Magnonic band structure, complete bandgap, and collective spin wave excitation in nanoscale two-dimensional magnonic crystals

International Nuclear Information System (INIS)

Kumar, D.; Barman, A.; Kłos, J. W.; Krawczyk, M.

2014-01-01

We present the observation of a complete bandgap and collective spin wave excitation in two-dimensional magnonic crystals comprised of arrays of nanoscale antidots and nanodots, respectively. Considering that the frequencies dealt with here fall in the microwave band, these findings can be used for the development of suitable magnonic metamaterials and spin wave based signal processing. We also present the application of a numerical procedure, to compute the dispersion relations of spin waves for any high symmetry direction in the first Brillouin zone. The results obtained from this procedure have been reproduced and verified by the well established plane wave method for an antidot lattice, when magnetization dynamics at antidot boundaries are pinned. The micromagnetic simulation based method can also be used to obtain iso–frequency contours of spin waves. Iso–frequency contours are analogous of the Fermi surfaces and hence, they have the potential to radicalize our understanding of spin wave dynamics. The physical origin of bands, partial and full magnonic bandgaps have been explained by plotting the spatial distribution of spin wave energy spectral density. Although, unfettered by rigid assumptions and approximations, which afflict most analytical methods used in the study of spin wave dynamics, micromagnetic simulations tend to be computationally demanding. Thus, the observation of collective spin wave excitation in the case of nanodot arrays, which can obviate the need to perform simulations, may also prove to be valuable

Spin selection at organic spinterface by anchoring group

Energy Technology Data Exchange (ETDEWEB)

Zhang, Zhao; Qiu, Shuai; Miao, Yuan-yuan; Ren, Jun-feng; Wang, Chuan-kui [School of Physics and Electronics, Shandong Normal University, Jinan 250014 (China); Hu, Gui-chao, E-mail: hgc@sdnu.edu.cn [School of Physics and Electronics, Shandong Normal University, Jinan 250014 (China); Institute of Theoretical Physics, Technische Universität Dresden, 01062 Dresden (Germany)

2017-07-01

Highlights: • The sign of interfacial spin polarization can be selected by using different anchoring groups. • A sp{sup 3}-d or sp-d hybridization may occur and induce spin polarization when the anchoring group changes. • Interfacial spin polarization depends on both the type of the outer orbital of the anchoring atom as well as its energy. - Abstract: Control of organic interfacial spin polarization is crucial in organic spintronics. Based on ab initio theory, here we proposed a spin selection at organic interface via anchoring group by adsorbing an organic molecule onto Ni(111) surface. The results demonstrate that either a positive or negative interfacial spin polarization may be obtained by choosing different anchoring groups. The orbital analysis via the projected density of states shows that the interfacial spin polarization is sensitive to the hybridization of the outer orbital of the anchoring atom as well as its energy relative to the d orbital of the ferromagnetic atom. The work indicates a feasible way to realize spin selection at the organic spinterface by anchoring group.

Optics with an Atom Laser Beam

International Nuclear Information System (INIS)

Bloch, Immanuel; Koehl, Michael; Greiner, Markus; Haensch, Theodor W.; Esslinger, Tilman

2001-01-01

We report on the atom optical manipulation of an atom laser beam. Reflection, focusing, and its storage in a resonator are demonstrated. Precise and versatile mechanical control over an atom laser beam propagating in an inhomogeneous magnetic field is achieved by optically inducing spin flips between atomic ground states with different magnetic moment. The magnetic force acting on the atoms can thereby be effectively switched on and off. The surface of the atom optical element is determined by the resonance condition for the spin flip in the inhomogeneous magnetic field. More than 98% of the incident atom laser beam is reflected specularly

Creating Spin-One Fermions in the Presence of Artificial Spin-Orbit Fields: Emergent Spinor Physics and Spectroscopic Properties

Science.gov (United States)

Kurkcuoglu, Doga Murat; de Melo, C. A. R. Sá

2018-05-01

We propose the creation and investigation of a system of spin-one fermions in the presence of artificial spin-orbit coupling, via the interaction of three hyperfine states of fermionic atoms to Raman laser fields. We explore the emergence of spinor physics in the Hamiltonian described by the interaction between light and atoms, and analyze spectroscopic properties such as dispersion relation, Fermi surfaces, spectral functions, spin-dependent momentum distributions and density of states. Connections to spin-one bosons and SU(3) systems is made, as well relations to the Lifshitz transition and Pomeranchuk instability are presented.

Quantum computation with nuclear spins in quantum dots

International Nuclear Information System (INIS)

Christ, H.

2008-01-01

The role of nuclear spins for quantum information processing in quantum dots is theoretically investigated in this thesis. Building on the established fact that the most strongly coupled environment for the potential electron spin quantum bit are the surrounding lattice nuclear spins interacting via the hyperfine interaction, we turn this vice into a virtue by designing schemes for harnessing this strong coupling. In this perspective, the ensemble of nuclear spins can be considered an asset, suitable for an active role in quantum information processing due to its intrinsic long coherence times. We present experimentally feasible protocols for the polarization, i.e. initialization, of the nuclear spins and a quantitative solution to our derived master equation. The polarization limiting destructive interference effects, caused by the collective nature of the nuclear coupling to the electron spin, are studied in detail. Efficient ways of mitigating these constraints are presented, demonstrating that highly polarized nuclear ensembles in quantum dots are feasible. At high, but not perfect, polarization of the nuclei the evolution of an electron spin in contact with the spin bath can be efficiently studied by means of a truncation of the Hilbert space. It is shown that the electron spin can function as a mediator of universal quantum gates for collective nuclear spin qubits, yielding a promising architecture for quantum information processing. Furthermore, we show that at high polarization the hyperfine interaction of electron and nuclear spins resembles the celebrated Jaynes-Cummings model of quantum optics. This result opens the door for transfer of knowledge from the mature field of quantum computation with atoms and photons. Additionally, tailored specifically for the quantum dot environment, we propose a novel scheme for the generation of highly squeezed collective nuclear states. Finally we demonstrate that even an unprepared completely mixed nuclear spin

Quantum computation with nuclear spins in quantum dots

Energy Technology Data Exchange (ETDEWEB)

Christ, H.

2008-01-24

The role of nuclear spins for quantum information processing in quantum dots is theoretically investigated in this thesis. Building on the established fact that the most strongly coupled environment for the potential electron spin quantum bit are the surrounding lattice nuclear spins interacting via the hyperfine interaction, we turn this vice into a virtue by designing schemes for harnessing this strong coupling. In this perspective, the ensemble of nuclear spins can be considered an asset, suitable for an active role in quantum information processing due to its intrinsic long coherence times. We present experimentally feasible protocols for the polarization, i.e. initialization, of the nuclear spins and a quantitative solution to our derived master equation. The polarization limiting destructive interference effects, caused by the collective nature of the nuclear coupling to the electron spin, are studied in detail. Efficient ways of mitigating these constraints are presented, demonstrating that highly polarized nuclear ensembles in quantum dots are feasible. At high, but not perfect, polarization of the nuclei the evolution of an electron spin in contact with the spin bath can be efficiently studied by means of a truncation of the Hilbert space. It is shown that the electron spin can function as a mediator of universal quantum gates for collective nuclear spin qubits, yielding a promising architecture for quantum information processing. Furthermore, we show that at high polarization the hyperfine interaction of electron and nuclear spins resembles the celebrated Jaynes-Cummings model of quantum optics. This result opens the door for transfer of knowledge from the mature field of quantum computation with atoms and photons. Additionally, tailored specifically for the quantum dot environment, we propose a novel scheme for the generation of highly squeezed collective nuclear states. Finally we demonstrate that even an unprepared completely mixed nuclear spin

Lamb shift and fine structure at n =2 in a hydrogenlike muonic atom with the nuclear spin I =0

Science.gov (United States)

Korzinin, Evgeny Yu.; Shelyuto, Valery A.; Ivanov, Vladimir G.; Karshenboim, Savely G.

2018-01-01

The paper is devoted to the Lamb shift and fine structure in a hydrogenlike muonic atom with a spinless nucleus up to the order α5m with all the recoil corrections included. Enhanced contributions of a higher order are also considered. We present the results on the pure QED contribution and on the finite-nuclear-size contribution, proportional to RN2, with the higher-order corrections included. We also consider the consistency of the pure QED theory and the evaluation of the nuclear-structure effects. Most of the QED theory is the same as the theory for the case of the nuclear spin 1/2. Additional nuclear-spin-dependent terms are considered in detail. The issue of the difference for the theories with a spinor nucleus and a scalar one is discussed for the recoil contributions in the order (Zα ) 4m ,α (Zα ) 4m , and (Zα ) 5m . The numerical results are presented for the muonic atoms with two lightest scalar nuclei, helium-4 and beryllium-10. We compare the theory of those muonic atoms with theory for the muonic hydrogen. Some higher-order finite-nuclear-size corrections for the Lamb shift in muonic hydrogen are revisited.

Homogenization of Doppler broadening in spin-noise spectroscopy

Science.gov (United States)

Petrov, M. Yu.; Ryzhov, I. I.; Smirnov, D. S.; Belyaev, L. Yu.; Potekhin, R. A.; Glazov, M. M.; Kulyasov, V. N.; Kozlov, G. G.; Aleksandrov, E. B.; Zapasskii, V. S.

2018-03-01

The spin-noise spectroscopy, being a nonperturbative linear optics tool, is still reputed to reveal a number of capabilities specific to nonlinear optics techniques. The effect of the Doppler broadening homogenization discovered in this work essentially widens these unique properties of spin-noise spectroscopy. We investigate spin noise of a classical system—cesium atoms vapor with admixture of buffer gas—by measuring the spin-induced Faraday rotation fluctuations in the region of D 2 line. The line, under our experimental conditions, is strongly inhomogeneously broadened due to the Doppler effect. Despite that, optical spectrum of the spin-noise power has the shape typical for the homogeneously broadened line with a dip at the line center. This fact is in stark contrast with the results of previous studies of inhomogeneous quantum dot ensembles and Doppler broadened atomic systems. In addition, the two-color spin-noise measurements have shown, in a highly spectacular way, that fluctuations of the Faraday rotation within the line are either correlated or anticorrelated depending on whether the two wavelengths lie on the same side or on different sides of the resonance. The experimental data are interpreted in the frame of the developed theoretical model which takes into account both kinetics and spin dynamics of Cs atoms. It is shown that the unexpected behavior of the Faraday rotation noise spectra and effective homogenization of the optical transition in the spin-noise measurements are related to smallness of the momentum relaxation time of the atoms as compared with their spin-relaxation time. Our findings demonstrate abilities of spin-noise spectroscopy for studying dynamic properties of inhomogeneously broadened ensembles of randomly moving spins.

The effects of spin in gases

International Nuclear Information System (INIS)

Laloee, F.; Freed, J.H.

1988-01-01

Low-density gases, in which atoms are separated by large distances, have long provided an enjoyable playground for physicists. One might suppose the pleasure of the playground would by now have been exhausted by the very simplicity of low-density gases. Recent work by a number of investigators including the author shows that this is not the case low-density gases continue to serve up a rich variety of phenomena as well as counterintuitive surprises. In particular, the macroscopic properties of a gas composed of individual hydrogen or helium atoms can under special circumstances by changed dramatically by quantum-mechanical effects. According to quantum theory, the nucleus of an atom behaves in a way similar to a rotating top, which has angular momentum about its axis of rotation; that is, the nucleus has spin, known more precisely as spin angular momentum. If the atoms of a gas are spin-polarized, so that their nuclei all have their spins pointing in the same direction, the viscosity of the gas can be changed enormously and so can its ability to conduct heat. Quantum-mechanical correlations among the nuclei called spin waves, which up to now had been observed only in certain liquids and solids such as magnets, can also arise. The changes are large enough for one to say the quantum-mechanical effects have caused the gas to take on entirely new properties. In a certain sense it is amazing to think that polarizing the nuclear spins can have any effect on the macroscopic properties of the gas, since the nuclear spins are son weakly coupled to the outside world. Yet the observations are in full agreement with with theory. Moreover, because spin-polarized gases are still fairly simple systems, they can be understood in terms fundamental principles, something that is still not possible to do in the case of liquids and solids

Few-particle quantum magnetism with ultracold atoms

Energy Technology Data Exchange (ETDEWEB)

Murmann, Simon

2015-11-25

This thesis reports on the deterministic preparation of magnetically ordered states in systems of few fermionic atoms. We follow the concept of quantum simulation and use {sup 6}Li atoms in two different hyperfine states to mimic the behavior of electrons in a solidstate system. In a first experiment, we simulate the two-site Hubbard model by using two atoms in an isolated double-well potential. We prepare the two-particle ground state of this model with a fidelity exceeding 90%. By introducing strong repulsive interactions, we are able to realize a pure spin model and describe the energy spectrum with a two-site Heisenberg Hamiltonian. In a second experiment, we realize Heisenberg spin chains of up to four atoms in a single strongly-elongated trapping potential. Here, the atoms self-align along the potential axis due to strong repulsive interactions. We introduce two novel measurement techniques to identify the state of the spin chains and thereby confirm that we can deterministically prepare antiferromagnetic ground-state systems. This constitutes the first observation of quantum magnetism with fermionic atoms that exceeds nearest-neighbor correlations. Both the double-well system and the spin chains can be seen as building blocks of larger ground-state spin systems. Their deterministic preparation therefore opens up a new bottom-up approach to the experimental realization of quantum many-body systems with ultracold atoms.

Search for Correlations between Prolate-Shape Collective and Oblate-Shape Non-Collective Nuclear Rotation: High Spin States in 159,160 Yb

International Nuclear Information System (INIS)

Byrski, T.; Beck, F.A.; Sharpey-Schafer, J.F.

1987-01-01

High-spin states of 159,160 Yb have been studied using the escape-suppressed array TESSA 2. Extensions of yrast and lateral bands have been found up to I ∼40. Experimental data suggest strong correlations between maximum alignment configurations of the valence nucleons and related collective states. Theoretical analysis fully supports the idea of prolate-collective vs. oblate-non-collective correlations. Band termination interpretation is discussed

Peculiarities of spin polarization inversion at a thiophene/cobalt interface

KAUST Repository

Wang, Xuhui

2013-03-20

We perform ab initio calculations to investigate the spin polarization at the interface between a thiophene molecule and cobalt substrate. We find that the reduced symmetry in the presence of a sulfur atom (in the thiophene molecule) leads to a strong spatial dependence of the spin polarization of the molecule. The two carbon atoms far from the sulfur acquire a polarization opposite to that of the substrate, while the carbon atoms bonded directly to sulfur possess the same polarization as the substrate. We determine the origin of this peculiar spin interface property as well as its impact on the spin transport.

Atomic physics

CERN Document Server

Born, Max

1969-01-01

The Nobel Laureate's brilliant exposition of the kinetic theory of gases, elementary particles, the nuclear atom, wave-corpuscles, atomic structure and spectral lines, electron spin and Pauli's principle, quantum statistics, molecular structure and nuclear physics. Over 40 appendices, a bibliography, numerous figures and graphs.

Many-body physics using cold atoms

Science.gov (United States)

Sundar, Bhuvanesh

Advances in experiments on dilute ultracold atomic gases have given us access to highly tunable quantum systems. In particular, there have been substantial improvements in achieving different kinds of interaction between atoms. As a result, utracold atomic gases oer an ideal platform to simulate many-body phenomena in condensed matter physics, and engineer other novel phenomena that are a result of the exotic interactions produced between atoms. In this dissertation, I present a series of studies that explore the physics of dilute ultracold atomic gases in different settings. In each setting, I explore a different form of the inter-particle interaction. Motivated by experiments which induce artificial spin-orbit coupling for cold fermions, I explore this system in my first project. In this project, I propose a method to perform universal quantum computation using the excitations of interacting spin-orbit coupled fermions, in which effective p-wave interactions lead to the formation of a topological superfluid. Motivated by experiments which explore the physics of exotic interactions between atoms trapped inside optical cavities, I explore this system in a second project. I calculate the phase diagram of lattice bosons trapped in an optical cavity, where the cavity modes mediates effective global range checkerboard interactions between the atoms. I compare this phase diagram with one that was recently measured experimentally. In two other projects, I explore quantum simulation of condensed matter phenomena due to spin-dependent interactions between particles. I propose a method to produce tunable spin-dependent interactions between atoms, using an optical Feshbach resonance. In one project, I use these spin-dependent interactions in an ultracold Bose-Fermi system, and propose a method to produce the Kondo model. I propose an experiment to directly observe the Kondo effect in this system. In another project, I propose using lattice bosons with a large hyperfine spin

High-precision measurement of the electron spin g factor of trapped atomic nitrogen in the endohedral fullerene N@C60

Science.gov (United States)

Wittmann, J. J.; Can, T. V.; Eckardt, M.; Harneit, W.; Griffin, R. G.; Corzilius, B.

2018-05-01

The electronic g factor carries highly useful information about the electronic structure of a paramagnetic species, such as spin-orbit coupling and dia- or paramagnetic (de-)shielding due to local fields of surrounding electron pairs. However, in many cases, a near "spin-only" case is observed, in particular for light elements, necessitating accurate and precise measurement of the g factors. Such measurement is typically impeded by a "chicken and egg situation": internal or external reference standards are used for relative comparison of electron paramagnetic resonance (EPR) Larmor frequencies. However, the g factor of the standard itself usually is subject to a significant uncertainty which directly limits the precision and/or accuracy of the sought after sample g factor. Here, we apply an EPR reference-free approach for determining the g factor of atomic nitrogen trapped within the endohedral fullerene C60:N@C60 in its polycrystalline state by measuring the 1H NMR resonance frequency of dispersing toluene at room temperature. We found a value of g = 2.00204 (4) with a finally reached relative precision of ∼20 ppm. This accurate measurement allows us to directly compare the electronic properties of N@C60 to those found in atomic nitrogen in the gas phase or trapped in other solid matrices at liquid helium temperature. We conclude that spin-orbit coupling in N@C60 at room temperature is very similar in magnitude and of same sign as found in other inert solid matrices and that interactions between the quartet spin system and the C60 molecular orbitals are thus negligible.

Elementary spin excitations in ultrathin itinerant magnets

Energy Technology Data Exchange (ETDEWEB)

Zakeri, Khalil, E-mail: zakeri@mpi-halle.de

2014-12-10

Elementary spin excitations (magnons) play a fundamental role in condensed matter physics, since many phenomena e.g. magnetic ordering, electrical (as well as heat) transport properties, ultrafast magnetization processes, and most importantly electron/spin dynamics can only be understood when these quasi-particles are taken into consideration. In addition to their fundamental importance, magnons may also be used for information processing in modern spintronics. Here the concept of spin excitations in ultrathin itinerant magnets is discussed and reviewed. Starting with a historical introduction, different classes of magnons are introduced. Different theoretical treatments of spin excitations in solids are outlined. Interaction of spin-polarized electrons with a magnetic surface is discussed. It is shown that, based on the quantum mechanical conservation rules, a magnon can only be excited when a minority electron is injected into the system. While the magnon creation process is forbidden by majority electrons, the magnon annihilation process is allowed instead. These fundamental quantum mechanical selection rules, together with the strong interaction of electrons with matter, make the spin-polarized electron spectroscopies as appropriate tools to excite and probe the elementary spin excitations in low-dimensional magnets e.g ultrathin films and nanostructures. The focus is put on the experimental results obtained by spin-polarized electron energy loss spectroscopy and spin-polarized inelastic tunneling spectroscopy. The magnon dispersion relation, lifetime, group and phase velocity measured using these approaches in various ultrathin magnets are discussed in detail. The differences and similarities with respect to the bulk excitations are addressed. The role of the temperature, atomic structure, number of atomic layers, lattice strain, electronic complexes and hybridization at the interfaces are outlined. A possibility of simultaneous probing of magnons and phonons

Experiments with a laser cooled cloud of atoms

International Nuclear Information System (INIS)

Natarajan, Vasant; Banerjee, Ayan; Rapol, Umakant

1999-01-01

We discuss two experiments that can be performed using a cloud of laser-cooled and trapped atoms, namely Bose-Einstein condensation (BEC) and search for a permanent Electric Dipole Moment (EDM). BEC can be observed in Rb atoms in a magnetic trap by using forced evaporative cooling to continuously lower the temperature below the condensation limit. The cloud is cooled by preferentially ejecting the hottest atoms from a magnetic trap. The magnetic trap is loaded with laser-cooled atoms from a magneto-optic trap. The EDM experiment can be performed with a laser-cooled cloud of Yb atoms. The atoms are spin polarized and the precession of the spin is measured in the presence of a strong electric field applied perpendicular to the spin direction. The use of laser-cooled atoms should greatly enhance the sensitivity of the experiment. (author)

Magnetism of one-dimensional strongly repulsive spin-1 bosons with antiferromagnetic spin-exchange interaction

International Nuclear Information System (INIS)

Lee, J. Y.; Guan, X. W.; Batchelor, M. T.; Lee, C.

2009-01-01

We investigate magnetism and quantum phase transitions in a one-dimensional system of integrable spin-1 bosons with strongly repulsive density-density interaction and antiferromagnetic spin-exchange interaction via the thermodynamic Bethe ansatz method. At zero temperature, the system exhibits three quantum phases: (i) a singlet phase of boson pairs when the external magnetic field H is less than the lower critical field H c1 ; (ii) a ferromagnetic phase of atoms in the hyperfine state |F=1, m F =1> when the external magnetic field exceeds the upper critical field H c2 ; and (iii) a mixed phase of singlet pairs and unpaired atoms in the intermediate region H c1 c2 . At finite temperatures, the spin fluctuations affect the thermodynamics of the model through coupling the spin bound states to the dressed energy for the unpaired m F =1 bosons. However, such spin dynamics is suppressed by a sufficiently strong external field at low temperatures. Thus the singlet pairs and unpaired bosons may form a two-component Luttinger liquid in the strong coupling regime.

mu. -nucleon atoms

Energy Technology Data Exchange (ETDEWEB)

Dobretsov, Yu; Dolgoshein, B; Kirillov-Ugryumov, V

1980-12-01

The properties and formation are described of ..mu..-nucleon atoms, the Larmor method of muon spin precession is discussed and the experimental confirmation of the existence of ..mu..-nucleon atoms is shown. The prospects of their use are indicated.

μ-nucleon atoms

International Nuclear Information System (INIS)

Dobretsov, Yu.; Dolgoshejn, B.; Kirillov-Ugryumov, V.

1980-01-01

The properties and formation are described of μ-nucleon atoms, the Larmor method of muon spin precession is discussed and the experimental confirmation of the existence of μ-nucleon atoms is shown. The prospects of their use are indicated. (J.P.)

Absence of a spin-signature from a single Ho adatom as probed by spin-sensitive tunneling.

Science.gov (United States)

Steinbrecher, M; Sonntag, A; dos Santos Dias, M; Bouhassoune, M; Lounis, S; Wiebe, J; Wiesendanger, R; Khajetoorians, A A

2016-02-03

Whether rare-earth materials can be used as single-atom magnetic memory is an ongoing debate in recent literature. Here we show, by inelastic and spin-resolved scanning tunnelling-based methods, that we observe a strong magnetic signal and excitation from Fe atoms adsorbed on Pt(111), but see no signatures of magnetic excitation or spin-based telegraph noise for Ho atoms. Moreover, we observe that the indirect exchange field produced by a single Ho atom is negligible, as sensed by nearby Fe atoms. We demonstrate, using ab initio methods, that this stems from a comparatively weak coupling of the Ho 4f electrons with both tunnelling electrons and substrate-derived itinerant electrons, making both magnetic coupling and detection very difficult when compared to 3d elements. We discuss these results in the context of ongoing disputes and clarify important controversies.

Effect of spin disorder on resistivity; Effet du desordre de spin sur la resistivite

Energy Technology Data Exchange (ETDEWEB)

Gennes, P.G. de [Commissariat a l' Energie Atomique, Saclay (France); Friedel, J [Faculte des Sciences de Paris, 75 (France)

1959-07-01

The resistivity of magnetic metals is studied in the case where the spin carriers are bound to the atoms (ex.: rare earths). The effect of short-range order is shown to be generally small even at the critical point. The inelasticity of the magnetic collisions between electrons and lattice can also be neglected, but this approximation becomes bad at low temperatures. In this region a spin-wave approximation is used. (author) [French] On etudie l'influence des phenomenes magnetiques sur la resistivite des metaux ou les porteurs de spin sont lies aux atomes (ex.: Terres rares). Une bonne approximation a temperature suffisamment elevee consiste a negliger l'ordre a courte distance et l'inelasticite des collisions magnetiques electrons-reseau. On montre que l'effet de l'ordre a courte distance est en general negligeable meme a la temperature critique. L'approximation devient fausse a basse temperature et doit alors etre remplacee par l'approximation des ondes de spin. (auteur)

Engineering hybrid Co-picene structures with variable spin coupling

Energy Technology Data Exchange (ETDEWEB)

Zhou, Chunsheng [Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026 (China); Department of Physics, University of Science and Technology of China, Hefei, Anhui 230026 (China); Shan, Huan; Li, Bin, E-mail: libin@mail.ustc.edu.cn, E-mail: adzhao@ustc.edu.cn; Zhao, Aidi, E-mail: libin@mail.ustc.edu.cn, E-mail: adzhao@ustc.edu.cn; Wang, Bing [Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026 (China)

2016-04-25

We report on the in situ engineering of hybrid Co-picene magnetic structures with variable spin coupling using a low-temperature scanning tunneling microscope. Single picene molecules adsorbed on Au(111) are manipulated to accommodate individual Co atoms one by one, forming stable artificial hybrid structures with magnetism introduced by the Co atoms. By monitoring the evolution of the Kondo effect at each site of Co atom, we found that the picene molecule plays an important role in tuning the spin coupling between individual Co atoms, which is confirmed by theoretical calculations based on the density-functional theory. Our findings indicate that the hybrid metal-molecule structures with variable spin coupling on surfaces can be artificially constructed in a controlled manner.

Collective spin correlations and entangled state dynamics in coupled quantum dots

Science.gov (United States)

Maslova, N. S.; Arseyev, P. I.; Mantsevich, V. N.

2018-02-01

Here we demonstrate that the dynamics of few-electron states in a correlated quantum-dot system coupled to an electronic reservoir is governed by the symmetry properties of the total system leading to the collective behavior of all the electrons. Time evolution of two-electron states in a correlated double quantum dot after coupling to the reservoir has been analyzed by means of kinetic equations for pseudoparticle occupation numbers with constraint on possible physical states. It was revealed that the absolute value of the spin correlation function and the degree of entanglement for two-electron states could considerably increase after coupling to the reservoir. The obtained results demonstrate the possibility of a controllable tuning of both the spin correlation function and the concurrence value in a coupled quantum-dot system by changing of the gate voltage applied to the barrier separating the dots.

Collective effects in spin polarized plasmas

International Nuclear Information System (INIS)

Coppi, B.; Cowley, S.; Detragiache, P.; Kulsrud, R.; Pegoraro, F.

1984-10-01

A fusing plasma with coherently polarized spin nuclei can be subject to instabilities due to the anisotropy of the reaction product distributions in velocity space, which is a result of their polarization. The characteristics of these instabilities depend strongly on the plasma spatial inhomogeneities and a significant rate of spin depolarization can be produced by them if adequate fluctuation amplitudes are reached. The results of the relevant analysis are, in addition, of interest for plasma heating processes with frequencies in the range of the cyclotron frequencies of the considered nuclei

Origin of spin-polarization in edge boron doped zigzag graphene nanoribbon: a potential spin filter.

Science.gov (United States)

Chakrabarty, Soubhik; Wasey, A H M Abdul; Thapa, Ranjit; Das, Gour Prasad

2018-06-04

To realize the graphene based spintronic device the prime challenge is to control the electronic structure of edges. In this work we find the origin of spin filtering property in edge boron doped zigzag graphene nanoribbon (ZGNRs) and provide a guide to prepare the graphene based next generation spin filter based device. Here we unveil the role of orbital (p-electron) to tune the electronic, magnetic and transport properties of the edge B doped ZGNRs. When all the edge carbon atoms at one of the edges of ZGNRs are replaced by B (100% edge B-doping), the system undergoes semiconductor to metal transition. The role of passivation of the edge with single/double atomic hydrogen on the electronic properties and its relation with the p electron is correlated in-depth. 50% edge B-doped ZGNRs (50% of the edge C atoms at one of the edges are replaced by B) also shows half-metallicity when the doped edge is left unpassivated. The half-metallic systems show 100% spin-filtering efficiency for a wide range of bias voltages. Zero bias transmission function of the other configurations shows asymmetric behavior for the up and down spin channels, thereby indicating their possible application potential in nano-spintronics. © 2018 IOP Publishing Ltd.

Quantum effects induced by a gap in the spectrum of atom-bath coupling constants: ''Freezing'' of atomic decay and monochromatic collective radiation

International Nuclear Information System (INIS)

Mogilevtsev, D.S.; Kilin, S.Ya.

1994-08-01

A specific kind of inhibition of atomic decay (''freezing of decay) and intense monochromatic collective radiation are predicted for a single two-level atom and for a system of atoms interacting with the field bath having the gap in the spectrum of coupling constants. (author). 10 refs, 5 figs

Max Auwaerter Price lecture: building and probing atomic structures

International Nuclear Information System (INIS)

Ternes, M.

2008-01-01

Full text: The control of the geometric, electronic, and magnetic properties of atomic-scale nanostructures is a prerequisite for the understanding and fabrication of new materials and devices. Two routes lead towards this goal: Atomic manipulation of single atoms and molecules by scanning probe microscopy, or patterning using self-assembly. Atomic manipulation has been performed since almost 20 years, but it has been difficult to answer the simple question: how much force does it take to manipulate atoms and molecules on surfaces? To address this question, we used a combined atomic force and scanning tunneling microscope to simultaneously measure the force and the current between an adsorbate and a tip during atomic manipulation. We found that the force it takes to move an atom depends crucially on the binding between adsorbate and surface. Our results indicate that for moving metal atoms on metal surfaces, the lateral force component plays the dominant role. Measuring the forces during manipulation yielded the full potential energy landscape of the tip-sample interaction. Surprisingly, the potential energy barriers are comparable to diffusion barriers, which are obtained in the absence of a probe tip. Furthermore, we used the scanning tunneling microscope to assemble magnetic structures on a thin insulator. We found, that the spin of the atom is influenced by the magnetocrystalline anisotropy of the supporting surface which lifts the spin degeneracy of the ground state and enables the identification of individual atoms. The ground state of atoms with half-integer spin remains always degenerated at zero field due to Kramers theorem. We found that if these states differ by an orbital momentum of m = ±1 the localized spin is screened by the surrounding conducting electrons of the non-magnetic host and form a many-electron spin-singlet at sufficiently low temperature. (author)

Topological Material-Based Spin Devices

Science.gov (United States)

Zhang, Minhao; Wang, Xuefeng

Three-dimensional topological insulators have insulating bulk and gapless helical surface states. One of the most fascinating properties of the metallic surface states is the spin-momentum helical locking. The giant current-driven torques on the magnetic layer have been discovered in TI/ferromagnet bilayers originating from the spin-momentum helical locking, enabling the efficient magnetization switching with a low current density. We demonstrated the current-direction dependent on-off state in TIs-based spin valve devices for memory and logic applications. Further, we demonstrated the Bi2Se3 system will go from a topologically nontrivial state to a topologically trivial state when Bi atoms are replaced by lighter In atoms. Here, topologically trivial metal (BixIny)2 Se3 with high mobility also facilitates the realization of its application in multifunctional spintronic devices.

Off-resonant transitions in the collective dynamics of multi-level atomic ensembles

DEFF Research Database (Denmark)

Miroshnychenko, Yevhen; Mølmer, Klaus

2013-01-01

We study the contributions of off-resonant transitions to the dynamics of a system of N multi-level atoms sharing one excitation and interacting with the quantized vector electromagnetic field. The rotating wave approximation significantly simplifies the derivation of the equations of motion...... describing the collective atomic dynamics, but it leads to an incorrect expression for the dispersive part of the atom–atom interaction terms. For the case of two-level atoms and a scalar electromagnetic field, it turns out that the atom–atom interaction can be recovered correctly if integrals over...... the photon mode frequencies are extended to incorporate negative values. We explicitly derive the atom–atom interaction for multi-level atoms, coupled to the full vector electromagnetic field, and we recover also in this general case the validity of the results obtained by the extension to negative...

Spin-glass transition in disordered terbium

International Nuclear Information System (INIS)

Hauser, J.J.

1985-01-01

While crystalline Tb is a helix antiferromagnet with a Neel temperature of 229 K which becomes ferromagnetic at 222 K, disordered Tb exhibits a spin-glass transition. The spin-glass freezing temperature ranges from 183 to 53 K, the lowest temperatures corresponding to the greatest degree of atomic disorder. These experiments constitute the first evidence for an elemental spin-glass. (author)

Theory of surface recombination of spin-polarized hydrogen

International Nuclear Information System (INIS)

Christou, C.T.; Haftel, M.I.

1989-01-01

A theory is presented, based on the Faddeev equations, for direct two-body recombination of hydrogen atoms on a liquid helium surface. The equations developed are applicable to hydrogen or deuterium atoms in any spin state, but are applied in particular to dipolar recombination of b state hydrogen atoms. The equations yield terms corresponding to one- and two-step processes. These terms are calculated for low temperatures (T = 0.1 to 1.1 K) and high field strengths (B = 4 to 14 T). The one-step term increases slowly with B, while the two-step term is rapidly decreasing. While the overall rate is quite small (∼5 x 10 -18 cm 2 /s) compared to recombination by two-body spin-relaxation, the results have important consequences in understanding the experimentally measured three-atom dipolar surface recombination rates. In three-atom recombination, where the role of spin-relaxation and the two-atom one-step processes are repressed, the role of the underlying two-atom, two-step process is enhanced. The field dependence of the process relevant to the three-atom system is calculated and found to be in fairly good agreement with the experimental three-atom data. The role of possible liquid excitations in enhancing the contribution of the two-step processes is also discussed. 33 refs.; 1 figure; 6 tabs

Spin injection into Pt-polymers with large spin-orbit coupling

Science.gov (United States)

Sun, Dali; McLaughlin, Ryan; Siegel, Gene; Tiwari, Ashutosh; Vardeny, Z. Valy

2014-03-01

Organic spintronics has entered a new era of devices that integrate organic light-emitting diodes (OLED) in organic spin valve (OSV) geometry (dubbed bipolar organic spin valve, or spin-OLED), for actively manipulating the device electroluminescence via the spin alignment of two ferromagnetic electrodes (Science 337, 204-209, 2012; Appl. Phys. Lett. 103, 042411, 2013). Organic semiconductors that contain heavy metal elements have been widely used as phosphorescent dopants in white-OLEDs. However such active materials are detrimental for OSV operation due to their large spin-orbit coupling (SOC) that may limit the spin diffusion length and thus spin-OLED based on organics with large SOC is a challenge. We report the successful fabrication of OSVs based on pi-conjugated polymers which contain intrachain Platinum atoms (dubbed Pt-polymers). Spin injection into the Pt-polymers is investigated by the giant magnetoresistance (GMR) effect as a function of bias voltage, temperature and polymer layer thickness. From the GMR bias voltage dependence we infer that the ``impendence mismatch'' between ferromagnetic electrodes and Pt-polymer may be suppressed due to the large SOC. Research sponsored by the NSF (Grant No. DMR-1104495) and NSF-MRSEC (DMR 1121252) at the University of Utah.

Spin crossover and high spin filtering behavior in Co-Pyridine and Co-Pyrimidine molecules

Science.gov (United States)

Wen, Zhongqian; Zhou, Liping; Cheng, Jue-Fei; Li, Shu-Jin; You, Wen-Long; Wang, Xuefeng

2018-03-01

We present a theoretical study on a series of cobalt complexes, which are constructed with cobalt atoms and pyridine/pyrimidine rings, using density functional theory. We investigate the structural and electric transport properties of spin crossover (SCO) Co complex with two spin states, namely low-spin configuration [LS] and high-spin configuration [HS]. Energy analyses of the two spin states imply that the SCO Co-Pyridine2 and Co-Pyrimidine2 complexes may display a spin transition process accompanied by a geometric modification driven by external stimuli. A nearly perfect spin filtering effect is observed in the Co-Pyrimidine2 complex with [HS] state. In addition, we also discover the contact-dependent transmission properties of Co-Pyridine2. These findings indicate that SCO Co complexes are promising materials for molecular spintronic devices.

Proton radioactivity at non-collective prolate shape in high spin state of 94Ag

International Nuclear Information System (INIS)

Aggarwal, Mamta

2010-01-01

We predict proton radioactivity and structural transitions in high spin state of an excited exotic nucleus near proton drip line in a theoretical framework and investigate the nature and the consequences of the structural transitions on separation energy as a function of temperature and spin. It reveals that the rotation of the excited exotic nucleus 94 Ag at excitation energies around 6.7 MeV and angular momentum near 21h generates a rarely seen prolate non-collective shape and proton separation energy becomes negative which indicates proton radioactivity in agreement with the experimental results of Mukha et al. for 94 Ag.

Spectrum of spin waves in cold polarized gases

Energy Technology Data Exchange (ETDEWEB)

Andreeva, T. L., E-mail: phdocandreeva@yandex.ru [Russian Academy of Sciences, Lebedev Physical Institute (Russian Federation)

2017-02-15

The spin dynamics of cold polarized gases are investigated using the Boltzmann equation. The dispersion relation for spin waves (transverse component of the magnetic moment) and the spin diffusion coefficient of the longitudinal component of the magnetic moment are calculated without using fitting parameters. The spin wave frequency and the diffusion coefficient for rubidium atoms are estimated numerically.

Laser resolution of unpolarized-electron scattering cross sections into spin-conserved and spin-flip components

International Nuclear Information System (INIS)

Ritchie, B.

1981-01-01

The theory is presented for one-photon free-free absorption by electrons scattering from high-Z atoms. The absorption cross section provides sufficient information to resolve the unpolarized-electron total cross section, Vertical Barf(theta)Vertical Bar 2 +Vertical Barg(theta)Vertical Bar 2 , into its individual components for spin-nonflip, Vertical Barf(theta)Vertical Bar 2 , and spin-flip, Vertical Barg(theta)Vertical Bar 2 , scattering. The observation of a spin-polarization effect for a spin-independent process (free-free absorption) is analogous to the Fano effect for bound-free absorption

NMRbot: Python scripts enable high-throughput data collection on current Bruker BioSpin NMR spectrometers.

Science.gov (United States)

Clos, Lawrence J; Jofre, M Fransisca; Ellinger, James J; Westler, William M; Markley, John L

2013-06-01

To facilitate the high-throughput acquisition of nuclear magnetic resonance (NMR) experimental data on large sets of samples, we have developed a simple and straightforward automated methodology that capitalizes on recent advances in Bruker BioSpin NMR spectrometer hardware and software. Given the daunting challenge for non-NMR experts to collect quality spectra, our goal was to increase user accessibility, provide customized functionality, and improve the consistency and reliability of resultant data. This methodology, NMRbot, is encoded in a set of scripts written in the Python programming language accessible within the Bruker BioSpin TopSpin ™ software. NMRbot improves automated data acquisition and offers novel tools for use in optimizing experimental parameters on the fly. This automated procedure has been successfully implemented for investigations in metabolomics, small-molecule library profiling, and protein-ligand titrations on four Bruker BioSpin NMR spectrometers at the National Magnetic Resonance Facility at Madison. The investigators reported benefits from ease of setup, improved spectral quality, convenient customizations, and overall time savings.

Modeling the collective excitations in a full Heusler Co2 FeAl0.5 Si0.5 (CFAS) spin valve magnetic nanopillar in the electromagnetic field

International Nuclear Information System (INIS)

David, Cherine; Arumugam, Brinda; Rajamani, Amuda; Natarajan, Kanimozhi

2014-01-01

This paper describes the physics of collective excitations that are caused by spin-transfer torques in CFAS magnetic multilayer. When the magnetizations of the pinned and free layers are not collinear with each other, the spin-polarized currents transfer angular momentum to the magnetizations near the interfaces, giving rise to spin-transfer torques. The currents in magnetic multilayer are spin polarised and can carry enough angular momentum. When an electron spin carried by the current interacts with a magnetic layer, the exchange interaction leads to torque between the spin and the magnetization vector of the free layer. This is Spin Transfer Torque (STT) and it excites the magnetization when it is large enough. The Spin Transfer Torque induced collective excitations for the CFAS spin valve pillar have been extensively studied in this paper. - Highlights: • We have modeled LLGS equation for CFAS multilayer array. • The dynamics of collective excitation induced by STT is investigated. • The interactions exhibit solitonic behaviour at both limiting modes of polarization. • The spin components of the solitons are graphically represented

Atomic Fermi-Bose mixtures in inhomogeneous and random lattices: From Fermi glass to quantum spin glass and quantum percolation

International Nuclear Information System (INIS)

Sanpera, A.; Lewenstein, M.; Kantian, A.; Sanchez-Palencia, L.; Zakrzewski, J.

2004-01-01

We investigate strongly interacting atomic Fermi-Bose mixtures in inhomogeneous and random optical lattices. We derive an effective Hamiltonian for the system and discuss its low temperature physics. We demonstrate the possibility of controlling the interactions at local level in inhomogeneous but regular lattices. Such a control leads to the achievement of Fermi glass, quantum Fermi spin-glass, and quantum percolation regimes involving bare and/or composite fermions in random lattices

X-ray laser implementation by means of a strong source of high-spin metastable atoms

International Nuclear Information System (INIS)

Helman, J.S.; Rau, C.; Bunge, C.F.

1983-01-01

High-spin metastable atomic beams of high density and extremely small divergence can be produced by electron capture during grazing-angle scattering of ion beams at ferromagnetic surfaces. This can be used to generate a long-lived reservoir of Li 1s2s2p 4 P/sub 5/2//sup ts0/ with enough density of metastables so that after laser-induced transfer to Li 1s2p/sup ts2/P strong lasing at 207 A should occur. This novel technique can also be used to produce a variety of other metastables known as potential candidates for lasing at shorter wavelengths

Inverse spin Hall effect from pulsed spin current in organic semiconductors with tunable spin-orbit coupling.

Science.gov (United States)

Sun, Dali; van Schooten, Kipp J; Kavand, Marzieh; Malissa, Hans; Zhang, Chuang; Groesbeck, Matthew; Boehme, Christoph; Valy Vardeny, Z

2016-08-01

Exploration of spin currents in organic semiconductors (OSECs) induced by resonant microwave absorption in ferromagnetic substrates is appealing for potential spintronics applications. Owing to the inherently weak spin-orbit coupling (SOC) of OSECs, their inverse spin Hall effect (ISHE) response is very subtle; limited by the microwave power applicable under continuous-wave (cw) excitation. Here we introduce a novel approach for generating significant ISHE signals in OSECs using pulsed ferromagnetic resonance, where the ISHE is two to three orders of magnitude larger compared to cw excitation. This strong ISHE enables us to investigate a variety of OSECs ranging from π-conjugated polymers with strong SOC that contain intrachain platinum atoms, to weak SOC polymers, to C60 films, where the SOC is predominantly caused by the curvature of the molecule's surface. The pulsed-ISHE technique offers a robust route for efficient injection and detection schemes of spin currents at room temperature, and paves the way for spin orbitronics in plastic materials.

Control of electron spin decoherence in nuclear spin baths

Science.gov (United States)

Liu, Ren-Bao

2011-03-01

Nuclear spin baths are a main mechanism of decoherence of spin qubits in solid-state systems, such as quantum dots and nitrogen-vacancy (NV) centers of diamond. The decoherence results from entanglement between the electron and nuclear spins, established by quantum evolution of the bath conditioned on the electron spin state. When the electron spin is flipped, the conditional bath evolution is manipulated. Such manipulation of bath through control of the electron spin not only leads to preservation of the center spin coherence but also demonstrates quantum nature of the bath. In an NV center system, the electron spin effectively interacts with hundreds of 13 C nuclear spins. Under repeated flip control (dynamical decoupling), the electron spin coherence can be preserved for a long time (> 1 ms) . Thereforesomecharacteristicoscillations , duetocouplingtoabonded 13 C nuclear spin pair (a dimer), are imprinted on the electron spin coherence profile, which are very sensitive to the position and orientation of the dimer. With such finger-print oscillations, a dimer can be uniquely identified. Thus, we propose magnetometry with single-nucleus sensitivity and atomic resolution, using NV center spin coherence to identify single molecules. Through the center spin coherence, we could also explore the many-body physics in an interacting spin bath. The information of elementary excitations and many-body correlations can be extracted from the center spin coherence under many-pulse dynamical decoupling control. Another application of the preserved spin coherence is identifying quantumness of a spin bath through the back-action of the electron spin to the bath. We show that the multiple transition of an NV center in a nuclear spin bath can have longer coherence time than the single transition does, when the classical noises due to inhomogeneous broadening is removed by spin echo. This counter-intuitive result unambiguously demonstrates the quantumness of the nuclear spin bath

Spin critical opalescence in zero-temperature Bose-Einstein condensates

Science.gov (United States)

Santamore, D. H.; Timmermans, E.

2012-02-01

Cold-atom developments suggest the prospect of measuring scaling properties and long-range fluctuations of continuous phase transitions at zero temperature. We discuss the conditions for characterizing the phase separation of Bose-Einstein condensates of boson atoms in two distinct hyperfine spin states. The mean-field description breaks down as the system approaches the transition from the miscible side. An effective spin description clarifies the ferromagnetic nature of the transition. We show that a difference in the scattering lengths for the bosons in the same spin state leads to an effective internal magnetic field. The point at which the internal magnetic field vanishes (i.e., equal values of the like-boson scattering lengths) is a special point. We show that the long-range density fluctuations are suppressed near that point, while the effective spin exhibits the long-range fluctuations that characterize critical points. The zero-temperature system exhibits critical opalescence with respect to long-wavelength waves of impurity atoms that interact with the bosons in a spin-dependent manner.

Coupling of spin and orbital motion of electrons in carbon nanotubes

DEFF Research Database (Denmark)

Kuemmeth, Ferdinand; Ilani, S; Ralph, D C

2008-01-01

Electrons in atoms possess both spin and orbital degrees of freedom. In non-relativistic quantum mechanics, these are independent, resulting in large degeneracies in atomic spectra. However, relativistic effects couple the spin and orbital motion, leading to the well-known fine structure in their...... systems, entailing new design principles for the realization of quantum bits (qubits) in nanotubes and providing a mechanism for all-electrical control of spins in nanotubes....

Survey of methods for rapid spin reversal

International Nuclear Information System (INIS)

McKibben, J.L.

1980-01-01

The need for rapid spin reversal technique in polarization experiments is discussed. The ground-state atomic-beam source equipped with two rf transitions for hydrogen can be reversed rapidly, and is now in use on several accelerators. It is the optimum choice provided the accelerator can accept H + ions. At present all rapid reversal experiments using H - ions are done with Lamb-shift sources; however, this is not a unique choice. Three methods for the reversal of the spin of the atomic beam within the Lamb-shift source are discussed in order of development. Coherent intensity and perhaps focus modulation seem to be the biggest problems in both types of sources. Methods for reducing these modulations in the Lamb-shift source are discussed. The same Lamb-shift apparatus is easily modified to provide information on the atomic physics of quenching of the 2S/sub 1/2/ states versus spin orientation, and this is also discussed. 2 figures

Joule heating and spin-transfer torque investigated on the atomic scale using a spin-polarized scanning tunneling microscope.

Science.gov (United States)

Krause, S; Herzog, G; Schlenhoff, A; Sonntag, A; Wiesendanger, R

2011-10-28

The influence of a high spin-polarized tunnel current onto the switching behavior of a superparamagnetic nanoisland on a nonmagnetic substrate is investigated by means of spin-polarized scanning tunneling microscopy. A detailed lifetime analysis allows for a quantification of the effective temperature rise of the nanoisland and the modification of the activation energy barrier for magnetization reversal, thereby using the nanoisland as a local thermometer and spin-transfer torque analyzer. Both the Joule heating and spin-transfer torque are found to scale linearly with the tunnel current. The results are compared to experiments performed on lithographically fabricated magneto-tunnel junctions, revealing a very high spin-transfer torque switching efficiency in our experiments.

Competition of multiplet and spin-orbit splitting in open-shells

Energy Technology Data Exchange (ETDEWEB)

Zhang, Qian; Koch, Erik [Institute for Advanced Simulation, Forschungszentrum Juelich (Germany)

2016-07-01

To study the trends in the spectra of open-shells across the periodic table, we perform density functional calculations for atoms and ions. We collect the Slater-Condon and spin-orbit parameters from the resulting self-consistent radial wave functions and potentials. To make these easily accessible, we provide a simple least squares fitting formula in the spirit of Slater's rules. Given these parameters we calculate the many-body spectra in LS-, intermediate-, and jj-coupling. To assess the relative importance of Coulomb and spin-orbit interactions, we estimate the width of the spectra by calculating the eigen-energy variance of the corresponding Hamiltonian using a simple formula that does not require diagonalizing a complicated many-body Hamiltonian.

Measuring the spin Chern number in time-reversal-invariant Hofstadter optical lattices

Energy Technology Data Exchange (ETDEWEB)

Zhang, Dan-Wei, E-mail: zdanwei@126.com [Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials, SPTE, South China Normal University, Guangzhou 510006 (China); Cao, Shuai, E-mail: shuaicao2004@163.com [Department of Applied Physics, College of Electronic Engineering, South China Agricultural University, Guangzhou 510642 China (China)

2016-10-14

We propose an experimental scheme to directly measure the spin Chern number of the time-reversal-invariant Hofstadter model in optical lattices. We first show that this model can be realized by using ultracold Fermi atoms with two pseudo-spin states encoded by the internal Zeeman states in a square optical lattice and the corresponding topological Bloch bands are characterized by the spin Chern number. We then propose and numerically demonstrate that this topological invariant can be extracted from the shift of the hybrid Wannier center in the optical lattice. By spin-resolved in situ detection of the atomic densities along the transverse direction combined with time-of-flight measurement along another spatial direction, the spin Chern number in this system is directly measured. - Highlights: • The cold-atom optical-lattice scheme for realizing the time-reversal-invariant Hofstadter model is proposed. • The intrinsic spin Chern number related to the hybrid Wannier center in the optical lattice is investigated. • Direct measurement of the spin Chern number in the proposed system is theoretically demonstrated.

Quasiparticle Breakdown in a Quantum Spin Liquid

International Nuclear Information System (INIS)

Stone, Matthew B.; Zalinznyak, I.; Hong, T.; Broholm, C.L.; Reich, D.H.

2006-01-01

Much of modern condensed matter physics is understood in terms of elementary excitations, or quasiparticles -- fundamental quanta of energy and momentum. Various strongly interacting atomic systems are successfully treated as a collection of quasiparticles with weak or no interactions. However, there are interesting limitations to this description: in some systems the very existence of quasiparticles cannot be taken for granted. Like unstable elementary particles, quasiparticles cannot survive beyond a threshold where certain decay channels become allowed by conservation laws; their spectrum terminates at this threshold. Such quasiparticle breakdown was first predicted for an exotic state of matter -- super-fluid 4 He at temperatures close to absolute zero, a quantum Bose liquid where zero-point atomic motion precludes crystallization. Here we show, using neutron scattering, that quasiparticle breakdown can also occur in a quantum magnet and, by implication, in other systems with Bose quasiparticles. We have measured spin excitations in a two-dimensional quantum magnet, piperazinium hexachlorodicuprate (PHCC), in which spin-1/2 copper ions form a non-magnetic quantum spin liquid, and find remarkable similarities with excitations in superfluid 4 He. We observe a threshold momentum beyond which the quasiparticle peak merges with the two-quasiparticle continuum. It then acquires a finite energy width and becomes indistinguishable from a leading-edge singularity, so that excited states are no longer quasiparticles but occupy a wide band of energy. Our findings have important ramifications for understanding excitations with gapped spectra in many condensed matter systems, ranging from band insulators to high-transition-temperature superconductors.

Spin currents and filtering behavior in zigzag graphene nanoribbons with adsorbed molybdenum chains

International Nuclear Information System (INIS)

García-Fuente, A; Gallego, L J; Vega, A

2015-01-01

By means of density-functional-theoretic calculations, we investigated the structural, electronic and transport properties of hydrogen-passivated zigzag graphene nanoribbons (ZGNRs) on which a one-atom-thick Mo chain was adsorbed (with or without one or two missing atoms), or in which the passivating hydrogen atoms were replaced by Mo atoms. Mo-passivated ZGNRs proved to be nonmagnetic. ZGNRs with an adsorbed defect-free Mo chain were most stable with the Mo atoms forming dimers above edge bay sites, which suppressed the magnetic moments of the C atoms in that half of the ribbon; around the Fermi level of these systems, each spin component had a transmission channel via the Mo sp z band and one had an additional channel created by polarization of the ZGNR π * band, leading to a net spin current. The absence of an Mo dimer from an Mo chain adsorbed at the ZGNR edge made the system a perfect spin filter at low voltage bias by suppressing the Mo sp z band channels. Thus this last kind of hybrid system is a potential spin valve. (paper)

Quantum group spin nets: Refinement limit and relation to spin foams

Science.gov (United States)

Dittrich, Bianca; Martin-Benito, Mercedes; Steinhaus, Sebastian

2014-07-01

So far spin foam models are hardly understood beyond a few of their basic building blocks. To make progress on this question, we define analogue spin foam models, so-called "spin nets," for quantum groups SU(2)k and examine their effective continuum dynamics via tensor network renormalization. In the refinement limit of this coarse-graining procedure, we find a vast nontrivial fixed-point structure beyond the degenerate and the BF phase. In comparison to previous work, we use fixed-point intertwiners, inspired by Reisenberger's construction principle [M. P. Reisenberger, J. Math. Phys. (N.Y.) 40, 2046 (1999)] and the recent work [B. Dittrich and W. Kaminski, arXiv:1311.1798], as the initial parametrization. In this new parametrization fine-tuning is not required in order to flow to these new fixed points. Encouragingly, each fixed point has an associated extended phase, which allows for the study of phase transitions in the future. Finally we also present an interpretation of spin nets in terms of melonic spin foams. The coarse-graining flow of spin nets can thus be interpreted as describing the effective coupling between two spin foam vertices or space time atoms.

Graphene nanoFlakes with large spin.

Science.gov (United States)

Wang, Wei L; Meng, Sheng; Kaxiras, Efthimios

2008-01-01

We investigate, using benzenoid graph theory and first-principles calculations, the magnetic properties of arbitrarily shaped finite graphene fragments to which we refer as graphene nanoflakes (GNFs). We demonstrate that the spin of a GNF depends on its shape due to topological frustration of the pi-bonds. For example, a zigzag-edged triangular GNF has a nonzero net spin, resembling an artificial ferrimagnetic atom, with the spin value scaling with its linear size. In general, the principle of topological frustration can be used to introduce large net spin and interesting spin distributions in graphene. These results suggest an avenue to nanoscale spintronics through the sculpting of graphene fragments.

Quantum phases of spinful Fermi gases in optical cavities

Science.gov (United States)

Colella, E.; Citro, R.; Barsanti, M.; Rossini, D.; Chiofalo, M.-L.

2018-04-01

We explore the quantum phases emerging from the interplay between spin and motional degrees of freedom of a one-dimensional quantum fluid of spinful fermionic atoms, effectively interacting via a photon-mediating mechanism with tunable sign and strength g , as it can be realized in present-day experiments with optical cavities. We find the emergence, in the very same system, of spin- and atomic-density wave ordering, accompanied by the occurrence of superfluidity for g >0 , while cavity photons are seen to drive strong correlations at all g values, with fermionic character for g >0 , and bosonic character for g analysis.

Spin-filter scanning tunneling microscopy : a novel technique for the analysis of spin polarization on magnetic surfaces and spintronic devices

NARCIS (Netherlands)

Vera Marun, I.J.

2010-01-01

This thesis deals with the development of a versatile technique to measure spin polarization with atomic resolution. A microscopy technique that can measure electronic spin polarization is relevant for characterization of magnetic nanostructures and spintronic devices. Scanning tunneling microscopy

Spin-interaction effects for ultralong-range Rydberg molecules in a magnetic field

Science.gov (United States)

Hummel, Frederic; Fey, Christian; Schmelcher, Peter

2018-04-01

We investigate the fine and spin structure of ultralong-range Rydberg molecules exposed to a homogeneous magnetic field. Each molecule consists of a 87Rb Rydberg atom the outer electron of which interacts via spin-dependent s - and p -wave scattering with a polarizable 87Rb ground-state atom. Our model includes also the hyperfine structure of the ground-state atom as well as spin-orbit couplings of the Rydberg and ground-state atom. We focus on d -Rydberg states and principal quantum numbers n in the vicinity of 40. The electronic structure and vibrational states are determined in the framework of the Born-Oppenheimer approximation for varying field strengths ranging from a few up to hundred Gauss. The results show that the interplay between the scattering interactions and the spin couplings gives rise to a large variety of molecular states in different spin configurations as well as in different spatial arrangements that can be tuned by the magnetic field. This includes relatively regularly shaped energy surfaces in a regime where the Zeeman splitting is large compared to the scattering interaction but small compared to the Rydberg fine structure, as well as more complex structures for both weaker and stronger fields. We quantify the impact of spin couplings by comparing the extended theory to a spin-independent model.

Effects of Rashba and Dresselhaus spin-orbit interactions on the ground state of two-dimensional localized spins.

Science.gov (United States)

Oh, J H; Lee, K-J; Lee, Hyun-Woo; Shin, M

2014-05-14

Starting with the indirect exchange model influenced by the Rashba and the Dresselhaus spin-orbit interactions, we derive the Dzyaloshinskii-Moriya interaction of localized spins. The strength of the Dzyaloshinskii-Moriya interaction is compared with that of the Heisenberg exchange term as a function of atomic distance. Using the calculated interaction strengths, we discuss the formation of various atomic ground states as a function of temperature and external magnetic field. By plotting the magnetic field-temperature phase diagram, we present approximate phase boundaries between the spiral, Skyrmion and ferromagnetic states of the two-dimensional weak ferromagnetic system.

QuSpin: a Python package for dynamics and exact diagonalisation of quantum many body systems part I: spin chains

Directory of Open Access Journals (Sweden)

Phillip Weinberg, Marin Bukov

2017-02-01

Full Text Available We present a new open-source Python package for exact diagonalization and quantum dynamics of spin(-photon chains, called QuSpin, supporting the use of various symmetries in 1-dimension and (imaginary time evolution for chains up to 32 sites in length. The package is well-suited to study, among others, quantum quenches at finite and infinite times, the Eigenstate Thermalisation hypothesis, many-body localisation and other dynamical phase transitions, periodically-driven (Floquet systems, adiabatic and counter-diabatic ramps, and spin-photon interactions. Moreover, QuSpin's user-friendly interface can easily be used in combination with other Python packages which makes it amenable to a high-level customisation. We explain how to use QuSpin using four detailed examples: (i Standard exact diagonalisation of XXZ chain (ii adiabatic ramping of parameters in the many-body localised XXZ model, (iii heating in the periodically-driven transverse-field Ising model in a parallel field, and (iv quantised light-atom interactions: recovering the periodically-driven atom in the semi-classical limit of a static Hamiltonian.

Inhibition of collective spontaneous decay and superradiance in an ensemble of sufficiently high quantity of excited identical atoms

International Nuclear Information System (INIS)

Basharov, A.M.

2011-01-01

New effects of suppression of the collective spontaneous emission and superradiance have been predicted. At a certain number N of ensemble atoms, the Stark interaction with a vacuum field was shown as being high enough for the excited N-atom ensemble to be stabilized with respect to the collective decay. The result was derived analytically as a consequence of applying the quantum stochastic differential equations to the description of the atomic dynamics in vacuum, where the Stark interaction operator is expressed in terms of the quantum Poisson process. -- Highlights: → Enhancement of the Stark interaction of N atoms ensemble with vacuum, with N rising. → Representation of the Stark interaction as the quantum Poisson process. → Collective spontaneous decay and superradiance under the strong Stark interaction. → Inhibition of superradiance at a certain number of ensemble atoms. → Analysis of superradiance experiments in terms of inhibition of collective decay.

Fast switching of bistable magnetic nanowires through collective spin reversal

Science.gov (United States)

Vindigni, Alessandro; Rettori, Angelo; Bogani, Lapo; Caneschi, Andrea; Gatteschi, Dante; Sessoli, Roberta; Novak, Miguel A.

2005-08-01

The use of magnetic nanowires as memory units is made possible by the exponential divergence of the characteristic time for magnetization reversal at low temperature, but the slow relaxation makes the manipulation of the frozen magnetic states difficult. We suggest that finite-size segments can show a fast switching if collective reversal of the spins is taken into account. This mechanism gives rise at low temperatures to a scaling law for the dynamic susceptibility that has been experimentally observed for the dilute molecular chain Co(hfac)2NitPhOMe. These results suggest a possible way of engineering nanowires for fast switching of the magnetization.

Spin-polarized 3He nuclear targets and metastable 4He atoms by optical pumping with a tunable, Nd:YAP laser

International Nuclear Information System (INIS)

Bohler, C.L.; Schearer, L.D.; Leduc, M.; Nacher, P.J.; Zachorowski, L.; Milner, R.G.; McKeown, R.D.; Woodward, C.E.

1988-01-01

Several Nd:YAP lasers were constructed which could be broadly tuned in the 1083-nm region which includes the helium 2 3 S-2 3 P transition, using a Lyot filter and thin, uncoated etalons within the laser cavity. 1 W of power could be extracted at 1083 nm through a 1% transmitting output coupler. This laser beam was used to optically pump metastable 4 He and 3 He 2 3 S helium atoms in a weak discharge cell, spin polarizing the metastable ensemble. In a 3 He cell the polarization is transferred to the nuclear spin system. A 3 He target cell at 0.3 Torr was polarized to 52% in a few minutes. We describe the application of this system to the design of polarized targets for experiments in nuclear physics

Rate equation modelling of the optically pumped spin-exchange source

International Nuclear Information System (INIS)

Stenger, J.; Rith, K.

1995-01-01

Sources for spin polarized hydrogen or deuterium, polarized via spin-exchange of a laser optically pumped alkali metal, can be modelled by rate equations. The rate equations for this type of source, operated either with hydrogen or deuterium, are given explicitly with the intention of providing a useful tool for further source optimization and understanding. Laser optical pumping of alkali metal, spin-exchange collisions of hydrogen or deuterium atoms with each other and with alkali metal atoms are included, as well as depolarization due to flow and wall collisions. (orig.)

Spin waves and spin instabilities in quantum plasmas

OpenAIRE

Andreev, P. A.; Kuz'menkov, L. S.

2014-01-01

We describe main ideas of method of many-particle quantum hydrodynamics allows to derive equations for description of quantum plasma evolution. We also present definitions of collective quantum variables suitable for quantum plasmas. We show that evolution of magnetic moments (spins) in quantum plasmas leads to several new branches of wave dispersion: spin-electromagnetic plasma waves and self-consistent spin waves. Propagation of neutron beams through quantum plasmas is also considered. Inst...

Spin polarized atom traps and fundamental symmetries

International Nuclear Information System (INIS)

Haeusser, O.

1994-10-01

Plans are described to couple a neutral atom trap to an upgraded version of TRIUMF's TISOL on-line mass separator. The unique properties of trapped and cooled atoms promise improvements of some symmetry tests of the Standard Model of the electroweak and strong interactions. (author). 33 refs., 3 figs

Spin-Lattice Coupling and Superconductivity in Fe Pnictides

Directory of Open Access Journals (Sweden)

T. Egami

2010-01-01

Full Text Available We consider strong spin-lattice and spin-phonon coupling in iron pnictides and discuss its implications on superconductivity. Strong magneto-volume effect in iron compounds has long been known as the Invar effect. Fe pnictides also exhibit this effect, reflected in particular on the dependence of the magnetic moment on the atomic volume of Fe defined by the positions of the nearest neighbor atoms. Through the phenomenological Landau theory, developed on the basis of the calculations by the density functional theory (DFT and the experimental results, we quantify the strength of the spin-lattice interaction as it relates to the Stoner criterion for the onset of magnetism. We suggest that the coupling between electrons and phonons through the spin channel may be sufficiently strong to be an important part of the superconductivity mechanism in Fe pnictides.

Spin valley and giant quantum spin Hall gap of hydrofluorinated bismuth nanosheet.

Science.gov (United States)

Gao, Heng; Wu, Wei; Hu, Tao; Stroppa, Alessandro; Wang, Xinran; Wang, Baigeng; Miao, Feng; Ren, Wei

2018-05-09

Spin-valley and electronic band topological properties have been extensively explored in quantum material science, yet their coexistence has rarely been realized in stoichiometric two-dimensional (2D) materials. We theoretically predict the quantum spin Hall effect (QSHE) in the hydrofluorinated bismuth (Bi 2 HF) nanosheet where the hydrogen (H) and fluorine (F) atoms are functionalized on opposite sides of bismuth (Bi) atomic monolayer. Such Bi 2 HF nanosheet is found to be a 2D topological insulator with a giant band gap of 0.97 eV which might host room temperature QSHE. The atomistic structure of Bi 2 HF nanosheet is noncentrosymmetric and the spontaneous polarization arises from the hydrofluorinated morphology. The phonon spectrum and ab initio molecular dynamic (AIMD) calculations reveal that the proposed Bi 2 HF nanosheet is dynamically and thermally stable. The inversion symmetry breaking together with spin-orbit coupling (SOC) leads to the coupling between spin and valley in Bi 2 HF nanosheet. The emerging valley-dependent properties and the interplay between intrinsic dipole and SOC are investigated using first-principles calculations combined with an effective Hamiltonian model. The topological invariant of the Bi 2 HF nanosheet is confirmed by using Wilson loop method and the calculated helical metallic edge states are shown to host QSHE. The Bi 2 HF nanosheet is therefore a promising platform to realize room temperature QSHE and valley spintronics.

Relativistic heavy-atom effects on heavy-atom nuclear shieldings

Science.gov (United States)

Lantto, Perttu; Romero, Rodolfo H.; Gómez, Sergio S.; Aucar, Gustavo A.; Vaara, Juha

2006-11-01

The principal relativistic heavy-atom effects on the nuclear magnetic resonance (NMR) shielding tensor of the heavy atom itself (HAHA effects) are calculated using ab initio methods at the level of the Breit-Pauli Hamiltonian. This is the first systematic study of the main HAHA effects on nuclear shielding and chemical shift by perturbational relativistic approach. The dependence of the HAHA effects on the chemical environment of the heavy atom is investigated for the closed-shell X2+, X4+, XH2, and XH3- (X =Si-Pb) as well as X3+, XH3, and XF3 (X =P-Bi) systems. Fully relativistic Dirac-Hartree-Fock calculations are carried out for comparison. It is necessary in the Breit-Pauli approach to include the second-order magnetic-field-dependent spin-orbit (SO) shielding contribution as it is the larger SO term in XH3-, XH3, and XF3, and is equally large in XH2 as the conventional, third-order field-independent spin-orbit contribution. Considering the chemical shift, the third-order SO mechanism contributes two-thirds of the difference of ˜1500ppm between BiH3 and BiF3. The second-order SO mechanism and the numerically largest relativistic effect, which arises from the cross-term contribution of the Fermi contact hyperfine interaction and the relativistically modified spin-Zeeman interaction (FC/SZ-KE), are isotropic and practically independent of electron correlation effects as well as the chemical environment of the heavy atom. The third-order SO terms depend on these factors and contribute both to heavy-atom shielding anisotropy and NMR chemical shifts. While a qualitative picture of heavy-atom chemical shifts is already obtained at the nonrelativistic level of theory, reliable shifts may be expected after including the third-order SO contributions only, especially when calculations are carried out at correlated level. The FC/SZ-KE contribution to shielding is almost completely produced in the s orbitals of the heavy atom, with values diminishing with the principal

Evolution of nuclear collectivity at high spins and temperatures

International Nuclear Information System (INIS)

Baktash, C.

1989-01-01

In the past few years, we have utilized the Spin Spectrometer and a variety of complementary probes (continuum γrays, proton-γ coincidence spectroscopy and γ decay of GDR) to study the nuclear response to the DIFFERENTIAL effects of increasing spin and temperature for constant values of excitation energy or spin, respectively. In this paper we shall describe two of the experiments that trace the properties of rapidly-rotating nuclei at small to moderate excitation energies. 22 refs., 7 figs

Proton radioactivity at non-collective prolate shape in high spin state of {sup 94}Ag

Energy Technology Data Exchange (ETDEWEB)

Aggarwal, Mamta, E-mail: mamta.a4@gmail.co [UM-DAE Centre for Excellence in Basic Sciences, University of Mumbai, Kalina Campus, Mumbai 400 098 (India)

2010-10-11

We predict proton radioactivity and structural transitions in high spin state of an excited exotic nucleus near proton drip line in a theoretical framework and investigate the nature and the consequences of the structural transitions on separation energy as a function of temperature and spin. It reveals that the rotation of the excited exotic nucleus {sup 94}Ag at excitation energies around 6.7 MeV and angular momentum near 21h generates a rarely seen prolate non-collective shape and proton separation energy becomes negative which indicates proton radioactivity in agreement with the experimental results of Mukha et al. for {sup 94}Ag.

Resonant quantum transitions in trapped antihydrogen atoms.

Science.gov (United States)

Amole, C; Ashkezari, M D; Baquero-Ruiz, M; Bertsche, W; Bowe, P D; Butler, E; Capra, A; Cesar, C L; Charlton, M; Deller, A; Donnan, P H; Eriksson, S; Fajans, J; Friesen, T; Fujiwara, M C; Gill, D R; Gutierrez, A; Hangst, J S; Hardy, W N; Hayden, M E; Humphries, A J; Isaac, C A; Jonsell, S; Kurchaninov, L; Little, A; Madsen, N; McKenna, J T K; Menary, S; Napoli, S C; Nolan, P; Olchanski, K; Olin, A; Pusa, P; Rasmussen, C Ø; Robicheaux, F; Sarid, E; Shields, C R; Silveira, D M; Stracka, S; So, C; Thompson, R I; van der Werf, D P; Wurtele, J S

2012-03-07

The hydrogen atom is one of the most important and influential model systems in modern physics. Attempts to understand its spectrum are inextricably linked to the early history and development of quantum mechanics. The hydrogen atom's stature lies in its simplicity and in the accuracy with which its spectrum can be measured and compared to theory. Today its spectrum remains a valuable tool for determining the values of fundamental constants and for challenging the limits of modern physics, including the validity of quantum electrodynamics and--by comparison with measurements on its antimatter counterpart, antihydrogen--the validity of CPT (charge conjugation, parity and time reversal) symmetry. Here we report spectroscopy of a pure antimatter atom, demonstrating resonant quantum transitions in antihydrogen. We have manipulated the internal spin state of antihydrogen atoms so as to induce magnetic resonance transitions between hyperfine levels of the positronic ground state. We used resonant microwave radiation to flip the spin of the positron in antihydrogen atoms that were magnetically trapped in the ALPHA apparatus. The spin flip causes trapped anti-atoms to be ejected from the trap. We look for evidence of resonant interaction by comparing the survival rate of trapped atoms irradiated with microwaves on-resonance to that of atoms subjected to microwaves that are off-resonance. In one variant of the experiment, we detect 23 atoms that survive in 110 trapping attempts with microwaves off-resonance (0.21 per attempt), and only two atoms that survive in 103 attempts with microwaves on-resonance (0.02 per attempt). We also describe the direct detection of the annihilation of antihydrogen atoms ejected by the microwaves.

Energies and damping rates of elementary excitations in spin-1 Bose-Einstein-condensed gases

International Nuclear Information System (INIS)

Szirmai, Gergely; Szepfalusy, Peter; Kis-Szabo, Krisztian

2003-01-01

The finite temperature Green's function technique is used to calculate the energies and damping rates of the elementary excitations of homogeneous, dilute, spin-1 Bose gases below the Bose-Einstein condensation temperature in both the density and spin channels. For this purpose a self-consistent dynamical Hartree-Fock model is formulated, which takes into account the direct and exchange processes on equal footing by summing up certain classes of Feynman diagrams. The model is shown to satisfy the Goldstone theorem and to exhibit the hybridization of one-particle and collective excitations correctly. The results are applied to gases of 23 Na and 87 Rb atoms

YBa{sub 2}Cu{sub 3}O{sub 7} microwave resonators for strong collective coupling with spin ensembles

Energy Technology Data Exchange (ETDEWEB)

Ghirri, A., E-mail: alberto.ghirri@nano.cnr.it [Istituto Nanoscienze - CNR, Centro S3, via Campi 213/a, 41125 Modena (Italy); Bonizzoni, C.; Affronte, M. [Dipartimento Fisica, Informatica e Matematica, Università di Modena e Reggio Emilia and Istituto Nanoscienze - CNR, Centro S3, via Campi 213/a, 41125 Modena (Italy); Gerace, D.; Sanna, S. [Dipartimento di Fisica, Università di Pavia, via Bassi 6, 27100 Pavia (Italy); Cassinese, A. [CNR-SPIN and Dipartimento di Fisica, Università di Napoli Federico II, 80138 Napoli (Italy)

2015-05-04

Coplanar microwave resonators made of 330 nm-thick superconducting YBa{sub 2}Cu{sub 3}O{sub 7} have been realized and characterized in a wide temperature (T, 2–100 K) and magnetic field (B, 0–7 T) range. The quality factor (Q{sub L}) exceeds 10{sup 4} below 55 K and it slightly decreases for increasing fields, remaining 90% of Q{sub L}(B=0) for B = 7 T and T = 2 K. These features allow the coherent coupling of resonant photons with a spin ensemble at finite temperature and magnetic field. To demonstrate this, collective strong coupling was achieved by using di(phenyl)-(2,4,6-trinitrophenyl)iminoazanium organic radical placed at the magnetic antinode of the fundamental mode: the in-plane magnetic field is used to tune the spin frequency gap splitting across the single-mode cavity resonance at 7.75 GHz, where clear anticrossings are observed with a splitting as large as ∼82 MHz at T = 2 K. The spin-cavity collective coupling rate is shown to scale as the square root of the number of active spins in the ensemble.

Magnetic Dichroism of Potassium Atoms on the Surface of Helium Nanodroplets

International Nuclear Information System (INIS)

Nagl, Johann; Auboeck, Gerald; Callegari, Carlo; Ernst, Wolfgang E.

2007-01-01

The population ratio of Zeeman sublevels of atoms on the surface of superfluid helium droplets (T=0.37 K) has been measured. Laser induced fluorescence spectra of K atoms are measured in the presence of a moderately strong magnetic field (2.9 kG). The relative difference between the two states of circular polarization of the exciting laser is used to determine the electron spin polarization of the ensemble. Equal fluorescence levels indicate that the two spin sublevels of the ground-state K atom are equipopulated, within 1%. Thermalization to 0.37 K would give a population ratio of 0.35. We deduce that the rate of spin relaxation induced by the droplet must be 2 triplet dimer we find instead full thermalization of the spin

Spin squeezing and entanglement in a dispersive cavity

International Nuclear Information System (INIS)

Deb, R. N.; Abdalla, M. Sebawe; Hassan, S. S.; Nayak, N.

2006-01-01

We consider a system of N two-level atoms (spins) interacting with the radiation field in a dispersive but high-Q cavity. Under an adiabatic condition, the interaction Hamiltonian reduces to a function of spin operators which is capable of producing spin squeezing. For a bipartite system (N=2), the expressions for spin squeezing get very simple, giving a clear indication of close to 100% noise reduction. We analyse this squeezing as a measure of bipartite entanglement

Lasing by driven atoms-cavity system in collective strong coupling regime.

Science.gov (United States)

Sawant, Rahul; Rangwala, S A

2017-09-12

The interaction of laser cooled atoms with resonant light is determined by the natural linewidth of the excited state. An optical cavity is another optically resonant system where the loss from the cavity determines the resonant optical response of the system. The near resonant combination of an optical Fabry-Pérot cavity with laser cooled and trapped atoms couples two distinct optical resonators via light and has great potential for precision measurements and the creation of versatile quantum optics systems. Here we show how driven magneto-optically trapped atoms in collective strong coupling regime with the cavity leads to lasing at a frequency red detuned from the atomic transition. Lasing is demonstrated experimentally by the observation of a lasing threshold accompanied by polarization and spatial mode purity, and line-narrowing in the outcoupled light. Spontaneous emission into the cavity mode by the driven atoms stimulates lasing action, which is capable of operating as a continuous wave laser in steady state, without a seed laser. The system is modeled theoretically, and qualitative agreement with experimentally observed lasing is seen. Our result opens up a range of new measurement possibilities with this system.

Anomalous tunneling of collective excitations and effects of superflow in the polar phase of a spin-1 spinor Bose-Einstein condensate

International Nuclear Information System (INIS)

Watabe, Shohei; Ohashi, Yoji; Kato, Yusuke

2011-01-01

We investigate tunneling properties of collective modes in the polar phase of a spin-1 spinor Bose-Einstein condensate (BEC). This spinor BEC state has two kinds of gapless modes (i.e., Bogoliubov and spin-wave). Within the framework of mean-field theory at T=0, we show that these Goldstone modes exhibit perfect transmission in the low-energy limit. Their anomalous tunneling behavior still holds in the presence of superflow, except in the critical current state. In the critical current state, while the tunneling of Bogoliubov mode is accompanied by finite reflection, the spin wave still exhibits perfect transmission, unless the strengths of spin-dependent and spin-independent interactions take the same value. We discuss the relation between perfect transmission of a spin wave and underlying superfluidity through a comparison of wave functions of the spin wave and the condensate.

Atomic probes of surface structure and dynamics

International Nuclear Information System (INIS)

Heller, E.J.; Jonsson, H.

1992-01-01

The following were studied: New semiclassical method for scattering calculations, He atom scattering from defective Pt surfaces, He atom scattering from Xe overlayers, thermal dissociation of H 2 on Cu(110), spin flip scattering of atoms from surfaces, and Car-Parrinello simulations of surface processes

Strong spin-filtering and spin-valve effects in a molecular V-C-60-V contact

DEFF Research Database (Denmark)

Koleini, Mohammad; Brandbyge, Mads

2012-01-01

Motivated by the recent achievements in the manipulation of C-60 molecules in STM experiments, we study theoretically the structure and electronic properties of a C-60 molecule in an STM tunneljunction with a magnetic tip and magnetic adatom on a Cu(111) surface using first-principles calculations....... For the case of a vanadium tip/adatom, we demonstrate how spin coupling between the magnetic V atoms, mediated by the C-60, can be observed in the electronic transport, which display a strong spin-filtering effect, allowing mainly majority-spin electrons to pass (>95%). Moreover, we find a significant change...... in the conductance between parallel and anti-parallel spin polarizations in the junction (86%) which suggests that STM experiments should be able to characterize the magnetism and spin coupling for these systems....

Density and spin linear response of atomic Fermi superfluids with population imbalance in the BCS–BEC crossover

International Nuclear Information System (INIS)

Guo, Hao; Li, Yang; He, Yan; Chien, Chih-Chun

2014-01-01

We present a theoretical study of the density and spin (representing the two components) linear response of Fermi superfluids with tunable attractive interactions and population imbalance. In both linear response theories, we find that the fluctuations of the order parameter must be treated on equal footing with the gauge transformations associated with the symmetries of the Hamiltonian so that important constraints including various sum rules can be satisfied. Both theories can be applied to the whole BCS–Bose–Einstein condensation crossover. The spin linear responses are qualitatively different with and without population imbalance because collective-mode effects from the fluctuations of the order parameter survive in the presence of population imbalance, even though the associated symmetry is not broken by the order parameter. Since a polarized superfluid becomes unstable at low temperatures in the weak and intermediate coupling regimes, we found that the density and spin susceptibilities diverge as the system approaches the unstable regime, but the emergence of phase separation preempts the divergence. (paper)

An approach to spin-resolved molecular gas microscopy

Science.gov (United States)

Covey, Jacob P.; De Marco, Luigi; Acevedo, Óscar L.; Rey, Ana Maria; Ye, Jun

2018-04-01

Ultracold polar molecules are an ideal platform for studying many-body physics with long-range dipolar interactions. Experiments in this field have progressed enormously, and several groups are pursuing advanced apparatus for manipulation of molecules with electric fields as well as single-atom-resolved in situ detection. Such detection has become ubiquitous for atoms in optical lattices and tweezer arrays, but has yet to be demonstrated for ultracold polar molecules. Here we present a proposal for the implementation of site-resolved microscopy for polar molecules, and specifically discuss a technique for spin-resolved molecular detection. We use numerical simulation of spin dynamics of lattice-confined polar molecules to show how such a scheme would be of utility in a spin-diffusion experiment.

On the electrodynamics of spinning particles

International Nuclear Information System (INIS)

Holten, J.W. van

1990-01-01

The electrodynamics of spinning point particles is considered. A modification of the Lorentz force law is introduced which can be interpreted as a classical limit of the Dirac-Klein-Gordon equation. An improved version of the inhomogeneous Maxwell equations is constructed to describe the classical fields of spinning particles. Both classical and quantum electrodynamics are shown to predict relativistic time-dilatation effects for spinning particles in an electromagnetic field, even in the limit of zero velocity. The life-time of unstable charged particles moving in a Coulomb field is computed for both spin-zero and spin-half particles. Comparison shows spin effects to be present but relatively small. The magnitude of further spin-dependent correction from hyperfine interactions is computed. A measurement of the life-time of muons in atomic bound states separated by such spin-dependent hyperfine interactions would provide a clean test for the effect predicted. Similar effects are shown to arise in non-abelian gauge theories such as QCD. (author). 18 refs

Amplitudes and state parameters from ion- and atom-atom excitation processes

International Nuclear Information System (INIS)

Andersen, T.; Horsdal-Pedersen, E.

1984-01-01

This chapter examines single collisions between two atomic species, one of which is initially in a 1 S state (there is only one initial spin channel). The collisions are characterized by a definite scattering plane and a definite orientation. Topics considered include an angular correlation between scattered particles and autoionization electrons or polarized photons emitted from states excited in atomic collisions (photon emission, electron emission, selectivity excited target atoms), experimental methods for obtaining information on the alignment and orientation parameters of atoms or ions excited in specific collisions, results of experiments and numerical calculations (quasi-oneelectron systems, He + -He collisions, other collision systems), and future aspects and possible applications of the polarizedphoton, scattered-particle coincidence techniques to atomic spectroscopy

Fragility of the fractional quantum spin Hall effect in quantum gases

International Nuclear Information System (INIS)

Fialko, O; Brand, J; Zülicke, U

2014-01-01

We consider the effect of contact interaction in a prototypical quantum spin Hall system of pseudo-spin-1/2 particles. A strong effective magnetic field with opposite directions for the two spin states restricts two-dimensional particle motion to the lowest Landau level. While interaction between same-spin particles leads to incompressible correlated states at fractional filling factors as known from the fractional quantum Hall effect, these states are destabilized by interactions between opposite spin particles. Exact results for two particles with opposite spin reveal a quasi-continuous spectrum of extended states with a large density of states at low energy. This has implications for the prospects of realizing the fractional quantum spin Hall effect in electronic or ultra-cold atom systems. Numerical diagonalization is used to extend the two-particle results to many bosonic particles and trapped systems. The interplay between an external trapping potential and spin-dependent interactions is shown to open up new possibilities for engineering exotic correlated many-particle states with ultra-cold atoms. (paper)

Dynamics of a driven spin coupled to an antiferromagnetic spin bath

International Nuclear Information System (INIS)

Yuan Xiaozhong; Goan, Hsi-Sheng; Zhu, Ka-Di

2011-01-01

We study the behavior of the Rabi oscillations of a driven central spin (qubit) coupled to an antiferromagnetic spin bath (environment). It is found that the decoherence behavior of the central spin depends on the detuning, driving strength, qubit-bath coupling and an important factor Ω, associated with the number of coupled atoms, the detailed lattice structure and the temperature of the environment. If detuning exists, Rabi oscillations may show the behavior of collapses and revivals; however, if detuning is absent, such a behavior will not appear. We investigate the weighted frequency distribution of the time evolution of the central spin inversion and give a reasonable explanation of this phenomenon of collapses and revivals. We also discuss the decoherence and pointer states of the qubit from the perspective of von Neumann entropy. We found that the eigenstates of the qubit self-Hamiltonian emerge as pointer states in the weak system-environment coupling limit.

Spin Filters as High-Performance Spin Polarimeters

International Nuclear Information System (INIS)

Rougemaille, N.; Lampel, G.; Peretti, J.; Drouhin, H.-J.; Lassailly, Y.; Filipe, A.; Wirth, T.; Schuhl, A.

2003-01-01

A spin-dependent transport experiment in which hot electrons pass through a ferromagnetic metal / semiconductor Schottky diode has been performed. A spin-polarized free-electron beam, emitted in vacuum from a GaAs photocathode, is injected into the thin metal layer with an energy between 5 and 1000 eV above to the Fermi level. The transmitted current collected in the semiconductor substrate increases with injection energy because of secondary - electron multiplication. The spin-dependent part of the transmitted current is first constant up to about 100 eV and then increases by 4 orders of magnitude. As an immediate application, the solid-state hybrid structure studied here leads to a very efficient and compact device for spin polarization detection

Laser optical pumping of sodium and lithium atom beams

International Nuclear Information System (INIS)

Cusma, J.T.

1983-01-01

The method of optical pumping with a continuous wave dye laser has been used to produce beams of polarized 23 Na atoms and polarized 6 Li atoms. Optical pumping of a 23 Na atom beam using either a multimode dye laser or a single frequency dye laser with a double passed acousto-optic modulator results in electron spin polarizations of 0.70-0.90 and nuclear spin polarizations of 0.75-0.90. Optical pumping of a 6 Li atom beam using a single frequency dye laser either with an acousto-optic modulator or with Doppler shift pumping results in electron spin polarizations of 0.77-0.95 and nuclear spin polarizations greater than 0.90. The polarization of the atom beam is measured using either the laser induced fluorescence in an intermediate magnetic field or a 6-pole magnet to determine the occupation probabilities of the ground hyperfine sublevels following optical pumping. The results of the laser optical pumping experiments agree with the results of a rate equation analysis of the optical pumping process which predicts that nearly all atoms are transferred into a single sublevel for our values of laser intensity and interaction time. The use of laser optical pumping in a polarized ion source for nuclear scattering experiments is discussed. The laser optical pumping method provides a means of constructing an intense source of polarized Li and Na ions

Quantum properties of spin polarized helium 3 optically oriented by a LNA laser

International Nuclear Information System (INIS)

Leduc, M.; Laloe, F.; Nacher, P.J.; Tastevin, G.; Daniels, J.M.; Betts, D.

1986-01-01

Spin polarized helium 3 (/sup 3/He increasing) and also atomic hydrogen (H decreasing) are systems exhibiting a number of unusual and interesting properties at low temperature. This is true even for dilute polarized gases in spite of the weakness of the nuclear magnetic interaction between atoms. The changes in the macroscopic properties of the gas with the nuclear polarization P are pure consequences of the indistinguishability of the particles and of the symmetrization principle in quantum mechanics. The transport properties of the gas, such as viscosity and thermal conductivity, have been calculated and found to be strongly dependent on P below a few kelvins. Spin transport in /sup 3/He increasing gives rise at low temperature to collective oscillatory modes: the transverse spin waves. Large changes are also expected with P in the case of more dense /sup 3/He fluids, such as an increase with P in the saturated vapor pressure. Optical pumping is a convenient technique for efficient polarization of the nuclear spins in /sup 3/He gas/sup 2/ making use of the 2/sup 3/S-2/sup 3/P atomic line at 1.08 μm. The arrival of cw tunable lasers in the near IR in the early 1980s gave a strong impulse to the buildup of experiments with a view to measuring quantum properties of /sup 3/He increasing at low temperature. Color center lasers (F/sup +//sub 2/ in NaF) provide P values up to 70%. They are now being replaced by more easy to handle LNA lasers which have given so far P in excess of 50% at room temperature. At low temperature, direct optical pumping of a /sup 3/He cell leads to poor P values; for that reason a different technique is used

Strong spin-filtering and spin-valve effects in a molecular V–C60–V contact

Directory of Open Access Journals (Sweden)

Mohammad Koleini

2012-08-01

Full Text Available Motivated by the recent achievements in the manipulation of C60 molecules in STM experiments, we study theoretically the structure and electronic properties of a C60 molecule in an STM tunneljunction with a magnetic tip and magnetic adatom on a Cu(111 surface using first-principles calculations. For the case of a vanadium tip/adatom, we demonstrate how spin coupling between the magnetic V atoms, mediated by the C60, can be observed in the electronic transport, which display a strong spin-filtering effect, allowing mainly majority-spin electrons to pass (>95%. Moreover, we find a significant change in the conductance between parallel and anti-parallel spin polarizations in the junction (86% which suggests that STM experiments should be able to characterize the magnetism and spin coupling for these systems.

Luther-Emery Phase and Atomic-Density Waves in a Trapped Fermion Gas

International Nuclear Information System (INIS)

Gao Xianlong; Rizzi, M.; Polini, Marco; Tosi, M. P.; Fazio, Rosario; Campo, V. L. Jr.; Capelle, K.

2007-01-01

The Luther-Emery liquid is a state of matter that is predicted to occur in one-dimensional systems of interacting fermions and is characterized by a gapless charge spectrum and a gapped spin spectrum. In this Letter we discuss a realization of the Luther-Emery phase in a trapped cold-atom gas. We study by means of the density-matrix renormalization-group technique a two-component atomic Fermi gas with attractive interactions subject to parabolic trapping inside an optical lattice. We demonstrate how this system exhibits compound phases characterized by the coexistence of spin pairing and atomic-density waves. A smooth crossover occurs with increasing magnitude of the atom-atom attraction to a state in which tightly bound spin-singlet dimers occupy the center of the trap. The existence of atomic-density waves could be detected in the elastic contribution to the light-scattering diffraction pattern

/sup 13/C-/sup 13/C spin-spin coupling constants in structural investigations. I. New method of determining the configuration of oximes and their derivatives

Energy Technology Data Exchange (ETDEWEB)

Krivdin, L.B.; Shcherbakov, V.V.; Kalabin, G.A.

1986-07-10

It was shown that the direct /sup 13/C-/sup 13/C spin-spin coupling constants can be used for the unambiguous identification of the configurational isomers of oximes and their derivatives. The stereospecificity of the constants is explained by the additional contribution from the unshared electron pair of the nitrogen atom to the spin-spin coupling constant between the adjacent carbon nuclei in the cis position.

Mott-insulating phases in unidimensional multi-components fermionic cold atoms

International Nuclear Information System (INIS)

Nonne, Heloise

2011-01-01

This thesis is devoted to the investigation of the Mott insulating phases arising in one-dimensional multicomponent fermionic cold atoms systems. The first part of this work is the study of a model with alkaline-earth cold atoms with nuclear spin I = 1/2. Those atoms enjoy an additional orbital degree of freedom, due to the presence of a metastable excited state; they thus have a total of four components. Our investigation is carried at half-filling, at strong and at weak couplings by means of analytic methods (conformal theory, bosonization, refermionization, renormalisation group). We found that the zero temperature phase diagram of the system is very rich: it contains seven Mott insulating phases, among which three are particularly interesting, since they display a hidden order, related to the Haldane physics of the antiferromagnetic spin-1 Heisenberg chain. Our conclusions are checked against numerical simulations, that were carried out with the density matrix renormalization group (DMRG) algorithm for intermediate couplings. The comparison shows an adiabatic continuity between the different regimes. A similar study for a model of cold atoms with hyperfine spin-3/2 highlights the Haldane physics in the charge sector of the degrees of freedom, with an effective model given by an antiferromagnetic pseudo-spin-1 chain. This analysis provides us an opportunity to investigate the zero temperature properties of the SO(5) bilinear-bi-quadratic Heisenberg chain. We show the presence of two gapped phases: one is dimerized, the other has a hidden symmetry (Z 2 x Z 2 ) 2 and spin-3/2 edge states, and they are separated by a critical point that belongs to the SO(5) 1 universality class. Finally, we investigate half-integer hyperfine spin cold atoms systems with 2N components which generalized the results obtained for the hyperfine spin-3/2 model. This leads us to find an even/odd effect according to the parity of N, very similar to the even/odd effect of spin chains

Dynamics of interacting fermions under spin-orbit coupling in an optical lattice clock

Science.gov (United States)

Bromley, S. L.; Kolkowitz, S.; Bothwell, T.; Kedar, D.; Safavi-Naini, A.; Wall, M. L.; Salomon, C.; Rey, A. M.; Ye, J.

2018-04-01

Quantum statistics and symmetrization dictate that identical fermions do not interact via s-wave collisions. However, in the presence of spin-orbit coupling (SOC), fermions prepared in identical internal states with distinct momenta become distinguishable. The resulting strongly interacting system can exhibit exotic topological and pairing behaviours, many of which are yet to be observed in condensed matter systems. Ultracold atomic gases offer a promising pathway for simulating these rich phenomena, but until recently have been hindered by heating and losses. Here we enter a new regime of many-body interacting SOC in a fermionic optical lattice clock (OLC), where the long-lived electronic clock states mitigate unwanted dissipation. Using clock spectroscopy, we observe the precession of the collective magnetization and the emergence of spin-locking effects arising from an interplay between p-wave and SOC-induced exchange interactions. The many-body dynamics are well captured by a collective XXZ spin model, which describes a broad class of condensed matter systems ranging from superconductors to quantum magnets. Furthermore, our work will aid in the design of next-generation OLCs by offering a route for avoiding the observed large density shifts caused by SOC-induced exchange interactions.

Universal Mechanism of Spin Relaxation in Solids

Science.gov (United States)

Chudnovsky, Eugene

2006-03-01

Conventional elastic theory ignores internal local twists and torques. Meantime, spin-lattice relaxation is inherently coupled with local elastic twists through conservation of the total angular momentum (spin + lattice). This coupling gives universal lower bound (free of fitting parameters) on the relaxation of the atomic or molecular spin in a solid [1] and on the relaxation of the electron spin in a quantum dot [2]. [1] E. M. Chudnovsky, D. A. Garanin, and R. Schilling, Phys. Rev. B 72, 094426 (2005). [2] C. Calero, E. M. Chudnovsky, and D. A. Garanin, Phys. Rev. Lett. 95, 166603 (2005).

Radio frequency scanning tunneling spectroscopy for single-molecule spin resonance.

Science.gov (United States)

Müllegger, Stefan; Tebi, Stefano; Das, Amal K; Schöfberger, Wolfgang; Faschinger, Felix; Koch, Reinhold

2014-09-26

We probe nuclear and electron spins in a single molecule even beyond the electromagnetic dipole selection rules, at readily accessible magnetic fields (few mT) and temperatures (5 K) by resonant radio-frequency current from a scanning tunneling microscope. We achieve subnanometer spatial resolution combined with single-spin sensitivity, representing a 10 orders of magnitude improvement compared to existing magnetic resonance techniques. We demonstrate the successful resonant spectroscopy of the complete manifold of nuclear and electronic magnetic transitions of up to ΔI(z)=±3 and ΔJ(z)=±12 of single quantum spins in a single molecule. Our method of resonant radio-frequency scanning tunneling spectroscopy offers, atom-by-atom, unprecedented analytical power and spin control with an impact on diverse fields of nanoscience and nanotechnology.

Robust Deterministic Controlled Phase-Flip Gate and Controlled-Not Gate Based on Atomic Ensembles Embedded in Double-Sided Optical Cavities

Science.gov (United States)

Liu, A.-Peng; Cheng, Liu-Yong; Guo, Qi; Zhang, Shou

2018-02-01

We first propose a scheme for controlled phase-flip gate between a flying photon qubit and the collective spin wave (magnon) of an atomic ensemble assisted by double-sided cavity quantum systems. Then we propose a deterministic controlled-not gate on magnon qubits with parity-check building blocks. Both the gates can be accomplished with 100% success probability in principle. Atomic ensemble is employed so that light-matter coupling is remarkably improved by collective enhancement. We assess the performance of the gates and the results show that they can be faithfully constituted with current experimental techniques.

Ab-initio investigation of spin-dependent transport properties in Fe-doped armchair graphyne nanoribbons

Energy Technology Data Exchange (ETDEWEB)

GolafroozShahri, S.; Roknabadi, M.R., E-mail: roknabad@um.ac.ir; Shahtahmasebi, N.; Behdani, M.

2016-12-15

An ab-initio study on the spin-polarized transport properties of H-passivated Fe-doped graphyne nanoribbons is presented. All the calculations were based on density functional theory (DFT). Doping single magnetic atom on graphyne nanoribbons leads to metallicity which can significantly improve the conductivity. The currents are not degenerate for both up and down spin electrons and they are considerably spin-polarized. Therefore a relatively good spin-filtering can be expected. For configurations with geometric symmetry spin-rectifying is also observed. Therefore they can be applied as a dual spin-filter or a dual spin-diode in spintronic equipment. - Highlights: • The existence of Fe additional electrons lead to metallicity. • Doping magnetic atom on studied n-AGyNRs, has improved the conductance of nanoribbons. • The current for both spin electrons is considerably spin-polarized. • Threshold voltage decreased by increasing the width of ribbon. • For configurations with geometric symmetry spin-rectifying effect was also observed.

Sources of polarized ions and atoms

International Nuclear Information System (INIS)

Cornelius, W.D.

1988-01-01

In this presentation we discuss methods of producing large quantities of polarized atoms and ions (Stern-Gerlach separation, optical pumping, and spin-exchange) as well as experimental methods of measuring the degree of polarization of atomic systems. The usefulness of polarized atoms in probing the microscopic magnetic surface properties of materials will also be discussed. 39 refs., 5 figs., 2 tabs

Internal spin structure of the nucleon

International Nuclear Information System (INIS)

Hughes, V.W.; Kuti, J.

1983-01-01

The study of the structure of the proton and neutron through deep inelastic scattering, initially with electrons but subsequently with muons and neutrinos as well, has played a central role in establishing the quark-parton theory of the composition of hadrons and of quantum chromodynamics (QCD). One important aspect of these theoretical and experimental developments is the two spin-dependent structure functions, which are independent of the two spin-averaged structure functions and define the internal spin structure of the nucleon. Since both quarks and gluons possess spin and the forces between them are spin dependent, we can expect important information on these forces and on nucleon structure to be obtained through the study of the spindependent aspects of the nucleon wave function, as has been the case before in atomic and nuclear physics

Quadrupole moments of low-lying baryons with spin- , spin- , and ...

Indian Academy of Sciences (India)

2013-02-03

Feb 3, 2013 ... boson (GB), successfully explains the 'proton spin crisis' [26], hyperon β decay parame- ters [27], strangeness content in the nucleon [28], and in the N ...... ment of India (SR/S2/HEP-0028/2008) and Department of Atomic Energy, Government of India (2010/37P/48/BRNS/1445). References. [1] R G Sachs ...

Investigation of non-collinear spin states with scanning tunneling microscopy.

Science.gov (United States)

Wulfhekel, W; Gao, C L

2010-03-05

Most ferromagnetic and antiferromagnetic substances show a simple collinear arrangement of the local spins. Under certain circumstances, however, the spin configuration is non-collinear. Scanning tunneling microscopy with its potential atomic resolution is an ideal tool for investigating these complex spin structures. Non-collinearity can be due to topological frustration of the exchange interaction, due to relativistic spin-orbit coupling or can be found in excited states. Examples for all three cases are given, illustrating the capabilities of spin-polarized scanning tunneling microscopy.

Interaction of relativistic elementary atoms with matter. I. General formulas

International Nuclear Information System (INIS)

Mrowczyn'ski, S.

1987-01-01

The problem of the interaction of relativistic elementary atoms (Coulomb bound states of elementary particles such as positronium, pionium, etc.) with matter is studied in the reference frame where the atom is initially at rest. An atom of matter is treated as a spinless structureless fast particle. The amplitudes of elementary-atom interaction are derived in the Born approximation under the assumption that a momentum transfer to the atom does not significantly exceed an inverse Bohr radius of the atom. The elementary-atom excitation and ionization processes are considered. The transitions where the spin projection of the atom component is reversed are also studied. In particular the matrix elements for para-ortho and ortho-para transitions are given. The spin structure of the amplitudes is discussed in detail. The sum rules, which allow the calculation of the cross sections summed over atom final states are found. Finally the formulas of the atom interaction cross sections are presented

Phase-space curvature in spin-orbit-coupled ultracold atomic systems

Science.gov (United States)

Armaitis, J.; Ruseckas, J.; Anisimovas, E.

2017-04-01

We consider a system with spin-orbit coupling and derive equations of motion which include the effects of Berry curvatures. We apply these equations to investigate the dynamics of particles with equal Rashba-Dresselhaus spin-orbit coupling in one dimension. In our derivation, the adiabatic transformation is performed first and leads to quantum Heisenberg equations of motion for momentum and position operators. These equations explicitly contain position-space, momentum-space, and phase-space Berry curvature terms. Subsequently, we perform the semiclassical approximation and obtain the semiclassical equations of motion. Taking the low-Berry-curvature limit results in equations that can be directly compared to previous results for the motion of wave packets. Finally, we show that in the semiclassical regime, the effective mass of the equal Rashba-Dresselhaus spin-orbit-coupled system can be viewed as a direct effect of the phase-space Berry curvature.

Understanding strong-field coherent control: Measuring single-atom versus collective dynamics

International Nuclear Information System (INIS)

Trallero-Herrero, Carlos; Weinacht, Thomas; Spanner, Michael

2006-01-01

We compare the results of two strong field coherent control experiments: one which optimizes multi-photon population transfer in atomic sodium (from the 3s to the 4s state, measured by spontaneous emission from the 3p-3s transition) with one that optimizes stimulated emission on the 3p-3s transition in an ensemble of sodium atoms. Both experiments make use of intense, shaped ultrafast laser pulses discovered by a Genetic Algorithm inside a learning control loop. Optimization leads to improvements in the spontaneous and stimulated emission yields of about 4 and 10 4 , respectively, over an unshaped pulse. We interpret these results by modeling both the single atom dynamics as well as the stimulated emission buildup through numerical integration of Schroedinger's and Maxwell's equations. Our interpretation leads to the conclusion that modest yields for controlling single quantum systems can lead to dramatic effects whenever an ensemble of such systems acts collectively following controlled impulsive excitation

Phenomena at very high spins

International Nuclear Information System (INIS)

Stephens, F.S.

1980-03-01

The present talk has three parts: first, a discussion of current ideas about the physics of very high spin states; second, some comments about noncollective behavior up to the highest spins where it is known, approx. 40 h; and finally, a presentation of the newest method for studying collective behavior up to spins of 60 to 70 h. The intention is that the overview presented in the first part will be sufficiently broad to indicate the relationship of the noncollective and collective behavior discussed in the other parts, and to provide some understanding of the compromise in behavior that seems to occur at the very highest spins. 13 figures

Spin-polarized gapped Dirac spectrum of unsupported silicene

Energy Technology Data Exchange (ETDEWEB)

Podsiadły-Paszkowska, A., E-mail: agata.podsiadly@gmail.com; Krawiec, M., E-mail: mariusz.krawiec@umcs.pl

2016-06-15

Highlights: • Effects of spin–orbit interaction and atomic reconstruction of silicene on its electronic properties have been studied. • Spin-polarized gapped Dirac spectrum has been revealed. • Two different AFM phases have been obtained. - Abstract: We study effects of the spin–orbit interaction and the atomic reconstruction of silicene on its electronic spectrum. As an example we consider unsupported silicene pulled off from Pb(111) substrate. Using first principles density functional theory we show that the inversion symmetry broken arrangement of atoms and the spin–orbit interaction generate a spin-polarized electronic spectrum with an energy gap in the Dirac cone. These findings are particularly interesting in view of the quantum anomalous and quantum valley Hall effects and should be observable in weakly interacting silicene-substrate systems.

Collective spin fluctuations in diluted magnetic semiconductors

Czech Academy of Sciences Publication Activity Database

König, J.; Schliemann, J.; Jungwirth, Tomáš; MacDonald, A. H.

2002-01-01

Roč. 12, - (2002), s. 379-382 ISSN 1386-9477 Institutional research plan: CEZ:AV0Z1010914 Keywords : spin fluctuation * magnetic semiconductors Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.107, year: 2002

Quantum quench in an atomic one-dimensional Ising chain.

Science.gov (United States)

Meinert, F; Mark, M J; Kirilov, E; Lauber, K; Weinmann, P; Daley, A J; Nägerl, H-C

2013-08-02

We study nonequilibrium dynamics for an ensemble of tilted one-dimensional atomic Bose-Hubbard chains after a sudden quench to the vicinity of the transition point of the Ising paramagnetic to antiferromagnetic quantum phase transition. The quench results in coherent oscillations for the orientation of effective Ising spins, detected via oscillations in the number of doubly occupied lattice sites. We characterize the quench by varying the system parameters. We report significant modification of the tunneling rate induced by interactions and show clear evidence for collective effects in the oscillatory response.

Influence of soliton distributions on the spin-dependent electronic ...

Indian Academy of Sciences (India)

interactions, so that spin memory can only be as long as a few seconds [6]. Therefore, spin-flip .... In addition, the term −σ · hβ is the internal exchange energy with hβ .... electrons density of states for short chains containing 100 carbon atoms.

Direct characterization of spin-transfer switching of nano-scale magnetic tunnel junctions using a conductive atomic force microscope

International Nuclear Information System (INIS)

Lee, Jia-Mou; Yang, Dong-Chin; Lee, Ching-Ming; Ye, Lin-Xiu; Chang, Yao-Jen; Wu, Te-ho; Lee, Yen-Chi; Wu, Jong-Ching

2013-01-01

We present an alternative method of spin-transfer-induced magnetization switching for magnetic tunnel junctions (MTJs) using a conductive atomic force microscope (CAFM) with pulsed current. The nominal MTJ cells' dimensions were 200 × 400 nm 2 . The AFM probes were coated with a Pt layer via sputtering to withstand up to several milliamperes. The pulsed current measurements, with pulse duration varying from 5 to 300 ms, revealed a magnetoresistance ratio of up to 120%, and an estimated intrinsic switching current density, based on the thermal activation model, of 3.94 MA cm −2 . This method demonstrates the potential skill to characterize nanometre-scale magnetic devices. (paper)

Spin microscope based on optically detected magnetic resonance

Science.gov (United States)

Berman, Gennady P.; Chernobrod, Boris M.

2007-12-11

The invention relates to scanning magnetic microscope which has a photoluminescent nanoprobe implanted in the tip apex of an atomic force microscope (AFM), a scanning tunneling microscope (STM) or a near-field scanning optical microscope (NSOM) and exhibits optically detected magnetic resonance (ODMR) in the vicinity of unpaired electron spins or nuclear magnetic moments in the sample material. The described spin microscope has demonstrated nanoscale lateral resolution and single spin sensitivity for the AFM and STM embodiments.

Spin transport in dangling-bond wires on doped H-passivated Si(100)

International Nuclear Information System (INIS)

Kepenekian, Mikaël; Robles, Roberto; Lorente, Nicolás; Rurali, Riccardo

2014-01-01

New advances in single-atom manipulation are leading to the creation of atomic structures on H-passivated Si surfaces with functionalities important for the development of atomic and molecular based technologies. We perform total-energy and electron-transport calculations to reveal the properties and understand the features of atomic wires crafted by H removal from the surface. The presence of dopants radically change the wire properties. Our calculations show that dopants have a tendency to approach the dangling-bond wires, and in these conditions, transport is enhanced and spin selective. These results have important implications in the development of atomic-scale spintronics showing that boron, and to a lesser extent phosphorous, convert the wires in high-quality spin filters. (paper)

Boson-mediated quantum spin simulators in transverse fields: X Y model and spin-boson entanglement

Science.gov (United States)

Wall, Michael L.; Safavi-Naini, Arghavan; Rey, Ana Maria

2017-01-01

The coupling of spins to long-wavelength bosonic modes is a prominent means to engineer long-range spin-spin interactions, and has been realized in a variety of platforms, such as atoms in optical cavities and trapped ions. To date, much of the experimental focus has been on the realization of long-range Ising models, but generalizations to other spin models are highly desirable. In this work, we explore a previously unappreciated connection between the realization of an X Y model by off-resonant driving of a single sideband of boson excitation (i.e., a single-beam Mølmer-Sørensen scheme) and a boson-mediated Ising simulator in the presence of a transverse field. In particular, we show that these two schemes have the same effective Hamiltonian in suitably defined rotating frames, and analyze the emergent effective X Y spin model through a truncated Magnus series and numerical simulations. In addition to X Y spin-spin interactions that can be nonperturbatively renormalized from the naive Ising spin-spin coupling constants, we find an effective transverse field that is dependent on the thermal energy of the bosons, as well as other spin-boson couplings that cause spin-boson entanglement not to vanish at any time. In the case of a boson-mediated Ising simulator with transverse field, we discuss the crossover from transverse field Ising-like to X Y -like spin behavior as a function of field strength.

Spin transport in oxygen adsorbed graphene nanoribbon

Science.gov (United States)

Kumar, Vipin

2018-04-01

The spin transport properties of pristine graphene nanoribbons (GNRs) have been most widely studied using theoretical and experimental tools. The possibilities of oxidation of fabricated graphene based nano electronic devices may change the device characteristics, which motivates to further explore the properties of graphene oxide nanoribbons (GONRs). Therefore, we present a systematic computational study on the spin polarized transport in surface oxidized GNR in antiferromagnetic (AFM) spin configuration using density functional theory combined with non-equilibrium Green's function (NEGF) method. It is found that the conductance in oxidized GNRs is significantly suppressed in the valance band and the conduction band. A further reduction in the conductance profile is seen in presence of two oxygen atoms on the ribbon plane. This change in the conductance may be attributed to change in the surface topology of the ribbon basal plane due to presence of the oxygen adatoms, where the charge transfer take place between the ribbon basal plane and the oxygen atoms.

Microfabricated Waveguide Atom Traps.

Energy Technology Data Exchange (ETDEWEB)

Jau, Yuan-Yu [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

2017-09-01

A nanoscale , microfabricated waveguide structure can in - principle be used to trap atoms in well - defined locations and enable strong photon-atom interactions . A neutral - atom platform based on this microfabrication technology will be prealigned , which is especially important for quantum - control applications. At present, there is still no reported demonstration of evanescent - field atom trapping using a microfabricated waveguide structure. We described the capabilities established by our team for future development of the waveguide atom - trapping technology at SNL and report our studies to overcome the technical challenges of loading cold atoms into the waveguide atom traps, efficient and broadband optical coupling to a waveguide, and the waveguide material for high - power optical transmission. From the atomic - physics and the waveguide modeling, w e have shown that a square nano-waveguide can be utilized t o achieve better atomic spin squeezing than using a nanofiber for first time.

Topological Phases in Graphene Nanoribbons: Junction States, Spin Centers, and Quantum Spin Chains

Science.gov (United States)

Cao, Ting; Zhao, Fangzhou; Louie, Steven G.

2017-08-01

We show that semiconducting graphene nanoribbons (GNRs) of different width, edge, and end termination (synthesizable from molecular precursors with atomic precision) belong to different electronic topological classes. The topological phase of GNRs is protected by spatial symmetries and dictated by the terminating unit cell. We have derived explicit formulas for their topological invariants and shown that localized junction states developed between two GNRs of distinct topology may be tuned by lateral junction geometry. The topology of a GNR can be further modified by dopants, such as a periodic array of boron atoms. In a superlattice consisting of segments of doped and pristine GNRs, the junction states are stable spin centers, forming a Heisenberg antiferromagnetic spin 1 /2 chain with tunable exchange interaction. The discoveries here not only are of scientific interest for studies of quasi-one-dimensional systems, but also open a new path for design principles of future GNR-based devices through their topological characters.

Electron--noble-gas spin-flip scattering at low energy

International Nuclear Information System (INIS)

Walker, T.G.; Bonin, K.; Happer, W.

1987-01-01

The spin-exchange rates and spin-relaxation rates for thermal electrons colliding with noble-gas atoms are calculated using the orthogonalized-plane-wave approximation and via partial-wave analysis. The two techniques give similar results and are in order-of-magnitude agreement with the experimental rate in Ar

On the Convergence of the ccJ-pVXZ and pcJ-n Basis Sets in CCSD Calculations of Nuclear Spin-Spin Coupling Constants

DEFF Research Database (Denmark)

Faber, Rasmus; Sauer, Stephan P. A.

2018-01-01

The basis set convergence of nuclear spin-spin coupling constants (SSCC) calculated at the coupled cluster singles and doubles (CCSD) level has been investigated for ten difficult molecules. Eight of the molecules contain fluorine atoms and nine contain double or triple bonds. Results obtained...

"Iron-Clad" Evidence For Spinning Black Hole

Science.gov (United States)

2003-09-01

Telltale X-rays from iron may reveal if black holes are spinning or not, according to astronomers using NASA's Chandra X-ray Observatory and the European Space Agency's XMM-Newton Observatory. The gas flows and bizarre gravitational effects observed near stellar black holes are similar to those seen around supermassive black holes. Stellar black holes, in effect, are convenient `scale models' of their much larger cousins. Black holes come in at least two different sizes. Stellar black holes are between five and 20 times the mass of the Sun. At the other end of the size scale, supermassive black holes contain millions or billions times the mass of our Sun. The Milky Way contains both a supermassive black hole at its center, as well as a number of stellar black holes sprinkled throughout the Galaxy. At a press conference at the "Four Years of Chandra" symposium in Huntsville, Ala., Jon Miller of the Harvard-Smithsonian Center for Astrophysics in Cambridge, Mass. discussed recent results on the X-ray spectra, or distribution of X-rays with energy, from the iron atoms in gas around three stellar black holes in the Milky Way. "Discovering the high degree of correspondence between stellar and supermassive black holes is a real breakthrough," said Miller. "Because stellar black holes are smaller, everything happens about a million times faster, so they can be used as a test-bed for theories of how spinning black holes affect the space and matter around them." X-rays from a stellar black hole are produced when gas from a nearby companion star is heated to tens of millions of degrees as it swirls toward the black hole. Iron atoms in this gas produce distinctive X-ray signals that can be used to study the orbits of particles around the black hole. For example, the gravity of a black hole can shift the X-rays to lower energies. "The latest work provides the most precise measurements yet of the X-ray spectra for stellar black holes," said Miller. "These data help rule out

Nuclear spin-spin coupling constants of linear carbon chains terminated by coronene molecules: a first principles study

International Nuclear Information System (INIS)

Oliveira, Joao Paulo Cavalcante; Mota, F. de Brito; Rivelino, Roberto

2011-01-01

Full text. Carbon nano wires made of long linear atomic chains have attracted considerable interest due to their potential applications in nano electronics. We report a density-functional-theory study of the nuclear spin-spin coupling constants for nano assemblies made of two coronene molecules bridged by carbon linear chains, considering distinct sizes and spin multiplicities. Also, we examine the effects of two terminal conformations (syn and anti) of the terminal anchor pieces on the magnetic properties of the carbon chains via 13 C NMR calculations. Our results reveal that simplified chemical models such as those based on cumulenes or polyynes are not appropriate to describe the linear chains with sp 2 terminations. For these types of atomic chains, the electronic ground state of the even-numbered chains can be singlet or triplet, whereas the ground state of the odd-numbered chains can be doublet or quartet. We discuss how the 13 C NMR chemical shift absorption is affected by increasing the size and changing the parity of the linear carbon chains. We have found that the J coupling constants between the carbon atoms in the linear chains present a well-defined pattern, in good accordance with our electronic structure calculations. For example, in the -C 4 - units we obtain couplings of 43.8, 114.5, 84.6, 114.5, and 43.8 Hz from one end to the other

Spin dynamics of large-spin fermions in a harmonic trap

Energy Technology Data Exchange (ETDEWEB)

Xu, Junjun; Feng, Tongtong; Gu, Qiang, E-mail: qgu@ustb.edu.cn

2017-04-15

Understanding the collective dynamics in a many-body system has been a central task in condensed matter physics. To achieve this task, we develop a Hartree–Fock theory to study the collective oscillations of spinor Fermi system, motivated by recent experiment on spin-9/2 fermions. We observe an oscillation period shoulder for small rotation angles. Different from previous studies, where the shoulder is found connected to the resonance from periodic to running phase, here the system is always in a running phase in the two-body phase space. This shoulder survives even in the many-body oscillations, which could be tested in the experiments. We also show how these collective oscillations evolve from two- to many-body. Our theory provides an alternative way to understand the collective dynamics in large-spin Fermi systems.

Efficient spin transitions in inelastic electron tunneling spectroscopy.

Science.gov (United States)

Lorente, Nicolás; Gauyacq, Jean-Pierre

2009-10-23

The excitation of the spin degrees of freedom of an adsorbed atom by tunneling electrons is computed using strong coupling theory. Recent measurements [Heinrich, Science 306, 466 (2004)] reveal that electron currents in a magnetic system efficiently excite its magnetic moments. Our theory shows that the incoming electron spin strongly couples with that of the adsorbate so that memory of the initial spin state is lost, leading to large excitation efficiencies. First-principles transmissions are evaluated in quantitative agreement with the experiment.

Variance squeezing and entanglement of the XX central spin model

International Nuclear Information System (INIS)

El-Orany, Faisal A A; Abdalla, M Sebawe

2011-01-01

In this paper, we study the quantum properties for a system that consists of a central atom interacting with surrounding spins through the Heisenberg XX couplings of equal strength. Employing the Heisenberg equations of motion we manage to derive an exact solution for the dynamical operators. We consider that the central atom and its surroundings are initially prepared in the excited state and in the coherent spin state, respectively. For this system, we investigate the evolution of variance squeezing and entanglement. The nonclassical effects have been remarked in the behavior of all components of the system. The atomic variance can exhibit revival-collapse phenomenon based on the value of the detuning parameter.

Variance squeezing and entanglement of the XX central spin model

Energy Technology Data Exchange (ETDEWEB)

El-Orany, Faisal A A [Department of Mathematics and Computer Science, Faculty of Science, Suez Canal University, Ismailia (Egypt); Abdalla, M Sebawe, E-mail: m.sebaweh@physics.org [Mathematics Department, College of Science, King Saud University PO Box 2455, Riyadh 11451 (Saudi Arabia)

2011-01-21

In this paper, we study the quantum properties for a system that consists of a central atom interacting with surrounding spins through the Heisenberg XX couplings of equal strength. Employing the Heisenberg equations of motion we manage to derive an exact solution for the dynamical operators. We consider that the central atom and its surroundings are initially prepared in the excited state and in the coherent spin state, respectively. For this system, we investigate the evolution of variance squeezing and entanglement. The nonclassical effects have been remarked in the behavior of all components of the system. The atomic variance can exhibit revival-collapse phenomenon based on the value of the detuning parameter.

Determination of the spin polarization of a 4He+ ion beam

International Nuclear Information System (INIS)

Suzuki, T.; Yamauchi, Y.

2008-01-01

It was demonstrated that the spin polarization of a 4 He + ion beam (P He + ) can be determined from the spin dependence of the electron emission in the deexcitation process of spin-polarized He metastable atoms (He*, 2 3 S 1 ) and spin-polarized He + ions on Fe (100) surfaces. On Fe (100) surfaces, both He* and He + deexcite via Auger neutralization, and therefore, the spin asymmetry obtained from spin-polarized He + ion neutralization spectroscopy should be equal to that from spin-polarized metastable He* deexcitation spectroscopy. The spin polarization of He* was obtained from Stern-Gerlach measurements. P He + was finally determined to be 0.19±0.02

Donor-driven spin relaxation in multivalley semiconductors.

Science.gov (United States)

Song, Yang; Chalaev, Oleg; Dery, Hanan

2014-10-17

The observed dependence of spin relaxation on the identity of the donor atom in n-type silicon has remained without explanation for decades and poses a long-standing open question with important consequences for modern spintronics. Taking into account the multivalley nature of the conduction band in silicon and germanium, we show that the spin-flip amplitude is dominated by short-range scattering off the central-cell potential of impurities after which the electron is transferred to a valley on a different axis in k space. Through symmetry arguments, we show that this spin-flip process can strongly affect the spin relaxation in all multivalley materials in which time-reversal cannot connect distinct valleys. From the physical insights gained from the theory, we provide guidelines to significantly enhance the spin lifetime in semiconductor spintronics devices.

Magnetism of a relaxed single atom vacancy in graphene

Science.gov (United States)

Wu, Yunyi; Hu, Yonghong; Xue, Li; Sun, Tieyu; Wang, Yu

2018-04-01

It has been suggested in literature that defects in graphene (e.g. absorbed atoms and vacancies) may induce magnetizations due to unpaired electrons. The nature of magnetism, i.e. ferromagnetic or anti-ferromagnetic, is dependent on a number of structural factors including locations of magnetic moments and lattice symmetry. In the present work we investigated the influence of a relaxed single atom vacancy in garphnene on magnetization which were obtained under different pinning boundary conditions, aiming to achieve a better understanding of the magnetic behaviors of graphene. Through first principles calculations, we found that major spin polarizations occur on atoms that deviate slightly from their original lattice positions, and pinning boundaries could also affect the relaxed positions of atoms and determine which atom(s) would become the main source(s) of total spin polarizations and magnetic moments. When the pinning boundary condition is free, a special non-magnetic and semi-conductive structure may be obtained, suggesting that magnetization should more readily occur under pinning boundary conditions.

Enhanced magnetoresistance in graphene spin valve

Energy Technology Data Exchange (ETDEWEB)

Iqbal, Muhammad Zahir, E-mail: zahir.upc@gmail.com [Faculty of Engineering Sciences, GIK Institute of Engineering Sciences and Technology, Topi 23640, Khyber Pakhtunkhwa (Pakistan); Hussain, Ghulam [Faculty of Engineering Sciences, GIK Institute of Engineering Sciences and Technology, Topi 23640, Khyber Pakhtunkhwa (Pakistan); Siddique, Salma [Department of Bioscience & Biotechnology, Sejong University, Seoul 143-747 (Korea, Republic of); Iqbal, Muhammad Waqas [Department of Physics, Riphah Institute of Computing and Applied Sciences (RICAS), Riphah International University, Lahore (Pakistan)

2017-05-01

Graphene has been explored as a promising candidate for spintronics due to its atomically flat structure and novel properties. Here we fabricate two spin valve junctions, one from directly grown graphene on Ni electrode (DG) and other from transferred graphene (TG). The magnetoresistance (MR) ratio for DG device is found to be higher than TG device i.e. ~0.73% and 0.14%, respectively. Also the spin polarization of Ni electrode is determined to be 6.03% at room temperature in case of DG device, however it reduces to 2.1% for TG device. From this analysis, we infer how environmental exposure of the sample degrades the spin properties of the magnetic junctions. Moreover, the transport measurements reveal linear behavior for current-voltage (I-V) characteristics, indicating ohmic behavior of the junctions. Our findings unveil the efficiency of direct growth of graphene for spin filtering mechanism in spin valve devices.

Electron spin resonance scanning tunneling microscope

International Nuclear Information System (INIS)

Guo Yang; Li Jianmei; Lu Xinghua

2015-01-01

It is highly expected that the future informatics will be based on the spins of individual electrons. The development of elementary information unit will eventually leads to novel single-molecule or single-atom devices based on electron spins; the quantum computer in the future can be constructed with single electron spins as the basic quantum bits. However, it is still a great challenge in detection and manipulation of a single electron spin, as well as its coherence and entanglement. As an ideal experimental tool for such tasks, the development of electron spin resonance scanning tunneling microscope (ESR-STM) has attracted great attention for decades. This paper briefly introduces the basic concept of ESR-STM. The development history of this instrument and recent progresses are reviewed. The underlying mechanism is explored and summarized. The challenges and possible solutions are discussed. Finally, the prospect of future direction and applications are presented. (authors)

Collective spin waves on a nanowire array with step-modulated thickness

International Nuclear Information System (INIS)

Gubbiotti, G; Tacchi, S; Kostylev, M; Ivanov, E; Samarin, S; Madami, M; Carlotti, G; Ding, J; Adeyeye, A O; Zighem, F; Stashkevich, A A

2014-01-01

It is shown experimentally that collective Bloch spin waves are able to propagate in a dense periodic array of nanowires with step-modulated thickness along the periodicity direction. The spin wave dispersion (frequency versus wave vector k) was measured using the Brillouin light scattering technique by sweeping the wave vector perpendicularly to the wire length. Remarkably, the mode measured at the lowest frequency exhibits an oscillating dispersion and its frequency is up-shifted with respect to the homogeneous-thickness wires of the same width. The modes located at higher frequencies have negligible dependencies on the wave number, i.e. are practically dispersionless. Complementary ferromagnetic resonance measurements enabled us to independently measure the whole set of modes at k = 0, showing a good agreement with the Brillouin light scattering data. These results have been successfully reproduced in a numerical simulation employing a two-dimensional Green's function description of the dynamic dipole field of the precessing magnetization. The theory also allowed visualizing the non-trivial distribution of dynamic magnetization across the wire cross-section and estimating the Brillouin light scattering cross-section. The analysis of these intensities suggests complicated magneto-optical coupling between the light and the dynamic magnetization in the arrays of nanowires with step-modulated thickness. This work can stimulate the design, tailoring, and characterization of three-dimensional magnonic crystals. (paper)

Phase transitions and spin excitations of spin-1 bosons in optical lattice

Science.gov (United States)

Zhu, Min-Jie; Zhao, Bo

2018-03-01

For spin-1 bosonic system trapped in optical lattice, we investigate two main problems, including MI-SF phase transition and magnetic phase separations in MI phase, with extended standard basis operator (SBO) method. For both ferromagnetic (U2 0) systems, we analytically figure out the symmetry properties in Mott-insulator and superfluid phases, which would provide a deeper insight into the MI-SF phase transition process. Then by applying self-consistent approach to the method, we include the effect of quantum and thermal fluctuations and derive the MI-SF transition phase diagram, which is in quantitative agreement with recent Monte-Carlo simulation at zero temperature, and at finite temperature, we find the underestimation of finite-temperature-effect in the mean-field approximation method. If we further consider the spin excitations in the insulating states of spin-1 system in external field, distinct spin phases are expected. Therefore, in the Mott lobes with n = 1 and n = 2 atoms per site, we give analytical and numerical boundaries of the singlet, nematic, partially magnetic and ferromagnetic phases in the magnetic phase diagrams.

Density profiles and collective excitations of a trapped two-component Fermi vapour

International Nuclear Information System (INIS)

Amoruso, M.; Meccoli, I.; Minguzzi, A.; Tosi, M.P.

1999-08-01

We discuss the ground state and the small-amplitude excitations of a degenerate vapour of fermionic atoms placed in two hyperfine states inside a spherical harmonic trap. An equations-of-motion approach is set up to discuss the hydrodynamic dissipation processes from the interactions between the two components of the fluid beyond mean-field theory and to emphasize analogies with spin dynamics and spin diffusion in a homogeneous Fermi liquid. The conditions for the establishment of a collisional regime via scattering against cold-atom impurities are analyzed. The equilibrium density profiles are then calculated for a two-component vapour of 40 K atoms: they are little modified by the interactions for presently relevant values of the system parameters, but spatial separation of the two components will spontaneously arise as the number of atoms in the trap is increased. The eigenmodes of collective oscillation in both the total particle number density and the concentration density are evaluated analytically in the special case of a symmetric two-component vapour in the collisional regime. The dispersion relation of the surface modes for the total particle density reduces in this case to that of a one-component Fermi vapour, whereas the frequencies of all other modes are shifted by the interactions. (author)

Quantum simulation of transverse Ising models with Rydberg atoms

Science.gov (United States)

Schauss, Peter

2018-04-01

Quantum Ising models are canonical models for the study of quantum phase transitions (Sachdev 1999 Quantum Phase Transitions (Cambridge: Cambridge University Press)) and are the underlying concept for many analogue quantum computing and quantum annealing ideas (Tanaka et al Quantum Spin Glasses, Annealing and Computation (Cambridge: Cambridge University Press)). Here we focus on the implementation of finite-range interacting Ising spin models, which are barely tractable numerically. Recent experiments with cold atoms have reached the interaction-dominated regime in quantum Ising magnets via optical coupling of trapped neutral atoms to Rydberg states. This approach allows for the tunability of all relevant terms in an Ising spin Hamiltonian with 1/{r}6 interactions in transverse and longitudinal fields. This review summarizes the recent progress of these implementations in Rydberg lattices with site-resolved detection. Strong correlations in quantum Ising models have been observed in several experiments, starting from a single excitation in the superatom regime up to the point of crystallization. The rapid progress in this field makes spin systems based on Rydberg atoms a promising platform for quantum simulation because of the unmatched flexibility and strength of interactions combined with high control and good isolation from the environment.

Parametric conversion and maximally entangled photon pair via collective excitations in a cycle atomic ensemble

International Nuclear Information System (INIS)

Li, J.; Yu, R.; Yang, X.

2008-01-01

We study the propagation of two quantized optical fields via considering the collective effects of photonic emissions and excitations of a three-level cyclic-type system (such as atomic ensemble with symmetry broken, or the chiral molecular gases, or manual 'atomic' array with symmetry broken), where the quantum transitions is driven by two quantized fields and a classical one. The results show that the parametric conversion and maximally entangled photon pair generation can be achieved by means of the collective excitation of the two upper energy levels induced by the classic optical field. This investigation may be used for the generated coherent short-wavelength quantum radiation and quantum information processing

Discovery of room-temperature spin-glass behaviors in two-dimensional oriented attached single crystals

Energy Technology Data Exchange (ETDEWEB)

Ma, Ji; Chen, Kezheng, E-mail: kchen@qust.edu.cn

2016-05-15

In this study, room-temperature spin-glass behaviors were observed in flake-like oriented attached hematite (α-Fe{sub 2}O{sub 3}) and iron phosphate hydroxide hydrate (Fe{sub 5}(PO{sub 4}){sub 4}(OH){sub 3}·2H{sub 2}O) single crystals. Remarkably, their coercivity (H{sub C}) values were found to be almost invariable at various given temperatures from 5 to 300 K. The spin topographic map in these flakes was assumed as superparamagnetic (SPM) “islands” isolated by spin glass (SG)-like “bridges”. A spin-glass model was then proposed to demonstrate the spin frustration within these “bridges”, which were formed by the staggered atomic planes in the uneven surfaces belonging to different attached nanoparticles. Under the spatial limitation and coupling shield of these “bridges”, the SPM “islands” were found to be collectively frozen to form a superspin glass (SSG) state below 80 K in weak applied magnetic fields; whereas, when strong magnetic fields were applied, the magnetic coupling of these “islands” would become superferromagnetic (SFM) through tunneling superexchange, so that, these SFM spins could antiferromagnetically couple with the SG-like “bridges” to yield pronounced exchange bias (EB) effect. - Highlights: • Room-temperature spin-glass state was found in 2D oriented attached single crystals. • Coercivity values were found to be almost invariable at different temperatures. • The spin topographic map was assumed as SPM “islands” isolated by SG-like “bridges”.

Spin glasses

CERN Document Server

Bovier, Anton

2007-01-01

Spin glass theory is going through a stunning period of progress while finding exciting new applications in areas beyond theoretical physics, in particular in combinatorics and computer science. This collection of state-of-the-art review papers written by leading experts in the field covers the topic from a wide variety of angles. The topics covered are mean field spin glasses, including a pedagogical account of Talagrand's proof of the Parisi solution, short range spin glasses, emphasizing the open problem of the relevance of the mean-field theory for lattice models, and the dynamics of spin glasses, in particular the problem of ageing in mean field models. The book will serve as a concise introduction to the state of the art of spin glass theory, usefull to both graduate students and young researchers, as well as to anyone curious to know what is going on in this exciting area of mathematical physics.

A high field optical-pumping spin-exchange polarized deuterium source

International Nuclear Information System (INIS)

Coulter, K.P.; Holt, R.J.; Kinney, E.R.; Kowalczyk, R.S.; Poelker, M.; Potterveld, D.H.; Young, L.; Zeidman, B.; Toporkov, D.

1992-01-01

Recent results from a prototype high field optical-pumping spin-exchange polarized deuterium source are presented. Atomic polarization as high as 62% have been observed with an intensity of 6.3 x 10 17 atoms-sec -1 and 65% dissociation fraction

Mechanical filter for alkali atoms

CERN Document Server

Toporkov, D K

2000-01-01

A device for separating gases of different mass is discussed. Such a device could be used in a laser-driven spin exchange source of polarized hydrogen atoms to reduce the contamination of alkali atoms. A Monte Carlo simulation has shown that the suggested apparatus based on a commercial turbo pump could reduce by a factor of 10-15 the concentration of the alkali-metal atoms in the hydrogen flow from a laser driven polarized source. This would greatly enhance the effective polarization in hydrogen targets.

Inducing spin-dependent tunneling to probe magnetic correlations in optical lattices

DEFF Research Database (Denmark)

Pedersen, Kim-Georg; Andersen, Brian; Syljuåsen, Olav

2012-01-01

We suggest a simple experimental method for probing antiferromagnetic spin correlations of two-component Fermi gases in optical lattices. The method relies on a spin selective Raman transition to excite atoms of one spin species to their first excited vibrational mode where the tunneling is large....... The resulting difference in the tunneling dynamics of the two spin species can then be exploited, to reveal the spin correlations by measuring the number of doubly occupied lattice sites at a later time. We perform quantum Monte Carlo simulations of the spin system and solve the optical lattice dynamics...

Spin-flip processes in low-energy Fe17+ + He collisions

International Nuclear Information System (INIS)

Bruch, R.; Altick, P.L.; Rauscher, E.; Wang, H.; Schneider, D.

1993-01-01

Spin-nonconserving electron transfer processes violating the ''Wigner rule'' have been studied for slow multiply charged ion-atom collisions. Experimentally a strong population of highly metastable sodium-like quartet states in low energy Fe 17+ + He single collision events has been observed. The possibility of double-electron capture plus spin-flip mechanisms has been discussed experimentally and theoretically, Our theoretical model using time dependent perturbation theory predicts that spin-flip processes are as likely as no spin flip under the conditions of our experiment

Picture change error in quasirelativistic electron/spin density, Laplacian and bond critical points

KAUST Repository

Bučinský , Luká š; Kucková , Lenka; Malček, Michal; Koží šek, Jozef; Biskupič, Stanislav; Jayatilaka, Dylan; Bü chel, Gabriel E.; Arion, Vladimir B.

2014-01-01

The change of picture of the quasirelativistic Hartree-Fock wave functions is considered for electron/spin densities, the negative Laplacian of electron density and the appropriate bond critical point characteristics from the Quantum Theory of Atoms In Molecules (QTAIM). [OsCl5(Hpz)]- and [RuCl5(NO)]2- transition metal complexes are considered. Both, scalar relativistic and spin-orbit effects have been accounted for using the Infinite Order Two Component (IOTC) Hamiltonian. Picture change error (PCE) correction in the electron and spin densities and the Laplacian of electron density are treated analytically. Generally, PCE is found significant only in the core region of the atoms for the electron/spin density as well as Laplacian.©2014 Elsevier B.V. All rights reserved.

Picture change error in quasirelativistic electron/spin density, Laplacian and bond critical points

KAUST Repository

Bučinský, Lukáš

2014-06-01

The change of picture of the quasirelativistic Hartree-Fock wave functions is considered for electron/spin densities, the negative Laplacian of electron density and the appropriate bond critical point characteristics from the Quantum Theory of Atoms In Molecules (QTAIM). [OsCl5(Hpz)]- and [RuCl5(NO)]2- transition metal complexes are considered. Both, scalar relativistic and spin-orbit effects have been accounted for using the Infinite Order Two Component (IOTC) Hamiltonian. Picture change error (PCE) correction in the electron and spin densities and the Laplacian of electron density are treated analytically. Generally, PCE is found significant only in the core region of the atoms for the electron/spin density as well as Laplacian.©2014 Elsevier B.V. All rights reserved.

Spin exchange in polarized deuterium

International Nuclear Information System (INIS)

Przewoski, B. von; Meyer, H.O.; Balewski, J.; Doskow, J.; Ibald, R.; Pollock, R.E.; Rinckel, T.; Wellinghausen, A.; Whitaker, T.J.; Daehnick, W.W.; Haeberli, W.; Schwartz, B.; Wise, T.; Lorentz, B.; Rathmann, F.; Pancella, P.V.; Saha, Swapan K.; Thoerngren-Engblom, P.

2003-01-01

We have measured the vector and tensor polarization of an atomic deuterium target as a function of the target density. The polarized deuterium was produced in an atomic beam source and injected into a storage cell. For this experiment, the atomic beam source was operated without rf transitions, in order to avoid complications from the unknown efficiency of these transitions. In this mode, the atomic beam is vector and tensor polarized and both polarizations can be measured simultaneously. We used a 1.2-cm-diam and 27-cm-long storage cell, which yielded an average target density between 3 and 9x10 11 at/cm 3 . We find that the tensor polarization decreases with increasing target density while the vector polarization remains constant. The data are in quantitative agreement with the calculated effect of spin exchange between deuterium atoms at low field

Controlling spin flips of molecules in an electromagnetic trap

Science.gov (United States)

Reens, David; Wu, Hao; Langen, Tim; Ye, Jun

2017-12-01

Doubly dipolar molecules exhibit complex internal spin dynamics when electric and magnetic fields are both applied. Near magnetic trap minima, these spin dynamics lead to enhancements in Majorana spin-flip transitions by many orders of magnitude relative to atoms and are thus an important obstacle for progress in molecule trapping and cooling. We conclusively demonstrate and address this with OH molecules in a trap geometry where spin-flip losses can be tuned from over 200 s-1 to below our 2 s-1 vacuum-limited loss rate with only a simple external bias coil and with minimal impact on trap depth and gradient.

Optically pumped electron spin polarized targets for use in the production of polarized ion beams

International Nuclear Information System (INIS)

Anderson, L.W.

1979-01-01

The production of relatively dense electron spin polarized alkali metal vapor targets by optical pumping with intense cw dye lasers is discussed. The target density and electron spin polarization depend on the dye laser intensity and bandwidth, the magnetic field at the target, and the electron spin depolarization time. For example in a magnetic field of 1.5 x 10 3 G, and using 1 W dye laser with a bandwidth of 10 10 Hz one can construct an electron spin polarized Na vapor target with a target thickness of 1.6 x 10 13 atoms/cm 2 and an average electron spin polarization of about 90% even though the Na atoms are completely depolarized at every wall collision. Possible uses of the electron spin polarized targets for the production of intense beams of polarized H - or 3 He - ions are discussed. (orig.)

Cellulose nanocrystal submonolayers by spin coating

NARCIS (Netherlands)

Kontturi, E.J.; Johansson, L.S.; Kontturi, K.S.; Ahonen, P.; Thune, P.C.; Laine, J.

2007-01-01

Dilute concentrations of cellulose nanocrystal solutions were spin coated onto different substrates to investigate the effect of the substrate on the nanocrystal submonolayers. Three substrates were probed: silica, titania, and amorphous cellulose. According to atomic force microscopy (AFM) images,

New insights into nano-magnetism by spin-polarized scanning tunneling microscopy

Energy Technology Data Exchange (ETDEWEB)

Sander, Dirk, E-mail: sander@mpi-halle.de [Max-Planck-Institut für Mikrostrukturphysik, Weinberg 2, D-06120 Halle/Saale (Germany); Oka, Hirofumi; Corbetta, Marco; Stepanyuk, Valeri; Kirschner, Jürgen [Max-Planck-Institut für Mikrostrukturphysik, Weinberg 2, D-06120 Halle/Saale (Germany)

2013-08-15

Highlights: ► We measure the magnetization reversal of individual nm small Co island by spin-STM. ► We identify an inhomogeneous magnetic anisotropy within a single Co island. ► The magnetic anisotropy near the rim is negligible as compared to 0.148 meV/atom at the island center. ► A crossover of the magnetization reversal from an exchange-spring behavior to domain wall formation is suggested. ► The impact of the observed spatial variation of the spin-dependent electronic properties on reversal is discussed. -- Abstract: We study the magnetization reversal and the position dependence of the spin-dependent electronic properties of nm small bilayer Co islands on Cu(1 1 1) by spin-polarized scanning tunneling microscopy in magnetic fields at low temperatures of 8 K. The analysis of the energy barrier of magnetization reversal from measurements of the switching field suggests a crossover of the magnetization reversal mode with increasing island size around 7500 atoms from exchange-spring behavior to domain wall formation. The quantitative analysis of the island size dependence of the energy barrier indicates an inhomogeneous magnetic anisotropy of the island. The island rim is magnetically soft, whereas the center shows a pronounced effective anisotropy of 0.148 meV/atom. We speculate that this inhomogeneity of the magnetic anisotropy might be a consequence of the spatial dependence of the spin-dependent electronic properties. We measure a spin-polarization and a tunnel magneto resistance ratio of opposite sign at the rim as compared to the island center.

New insights into nano-magnetism by spin-polarized scanning tunneling microscopy

International Nuclear Information System (INIS)

Sander, Dirk; Oka, Hirofumi; Corbetta, Marco; Stepanyuk, Valeri; Kirschner, Jürgen

2013-01-01

Highlights: ► We measure the magnetization reversal of individual nm small Co island by spin-STM. ► We identify an inhomogeneous magnetic anisotropy within a single Co island. ► The magnetic anisotropy near the rim is negligible as compared to 0.148 meV/atom at the island center. ► A crossover of the magnetization reversal from an exchange-spring behavior to domain wall formation is suggested. ► The impact of the observed spatial variation of the spin-dependent electronic properties on reversal is discussed. -- Abstract: We study the magnetization reversal and the position dependence of the spin-dependent electronic properties of nm small bilayer Co islands on Cu(1 1 1) by spin-polarized scanning tunneling microscopy in magnetic fields at low temperatures of 8 K. The analysis of the energy barrier of magnetization reversal from measurements of the switching field suggests a crossover of the magnetization reversal mode with increasing island size around 7500 atoms from exchange-spring behavior to domain wall formation. The quantitative analysis of the island size dependence of the energy barrier indicates an inhomogeneous magnetic anisotropy of the island. The island rim is magnetically soft, whereas the center shows a pronounced effective anisotropy of 0.148 meV/atom. We speculate that this inhomogeneity of the magnetic anisotropy might be a consequence of the spatial dependence of the spin-dependent electronic properties. We measure a spin-polarization and a tunnel magneto resistance ratio of opposite sign at the rim as compared to the island center

Laser method of free atom nuclei orientation

International Nuclear Information System (INIS)

Barabanov, A.L.

1987-01-01

Orientation process of free atom (atoms in beams) nuclei, scattering quanta of circularly polarized laser radiation is considered. A method for the evaluation of nuclei orientation parameters is developed. It is shown that in the process of pumping between the ground and first excited atomic states with electron shell spins J 1 and J 2 , so that J 2 = J 1 + 1, a complete orientation of nuclei can be attained

An endohedral fullerene-based nuclear spin quantum computer

International Nuclear Information System (INIS)

Ju Chenyong; Suter, Dieter; Du Jiangfeng

2011-01-01

We propose a new scalable quantum computer architecture based on endohedral fullerene molecules. Qubits are encoded in the nuclear spins of the endohedral atoms, which posses even longer coherence times than the electron spins which are used as the qubits in previous proposals. To address the individual qubits, we use the hyperfine interaction, which distinguishes two modes (active and passive) of the nuclear spin. Two-qubit quantum gates are effectively implemented by employing the electronic dipolar interaction between adjacent molecules. The electron spins also assist in the qubit initialization and readout. Our architecture should be significantly easier to implement than earlier proposals for spin-based quantum computers, such as the concept of Kane [B.E. Kane, Nature 393 (1998) 133]. - Research highlights: → We propose an endohedral fullerene-based scalable quantum computer architecture. → Qubits are encoded on nuclear spins, while electron spins serve as auxiliaries. → Nuclear spins are individually addressed using the hyperfine interaction. → Two-qubit gates are implemented through the medium of electron spins.

Trapped atoms along nanophotonic resonators

Science.gov (United States)

Fields, Brian; Kim, May; Chang, Tzu-Han; Hung, Chen-Lung

2017-04-01

Many-body systems subject to long-range interactions have remained a very challenging topic experimentally. Ultracold atoms trapped in extreme proximity to the surface of nanophotonic structures provides a dynamic system combining the strong atom-atom interactions mediated by guided mode photons with the exquisite control implemented with trapped atom systems. The hybrid system promises pair-wise tunability of long-range interactions between atomic pseudo spins, allowing studies of quantum magnetism extending far beyond nearest neighbor interactions. In this talk, we will discuss our current status developing high quality nanophotonic ring resonators, engineered on CMOS compatible optical chips with integrated nanostructures that, in combination with a side illuminating beam, can realize stable atom traps approximately 100nm above the surface. We will report on our progress towards loading arrays of cold atoms near the surface of these structures and studying atom-atom interaction mediated by photons with high cooperativity.

/sup 13/C-/sup 13/C spin-spin coupling constants in structural investigations. II. Conformational structure of vinyl ethers

Energy Technology Data Exchange (ETDEWEB)

Krivdin, L.B.; Shcherbakov, V.V.; Bzhezovskii, V.M.; Kalabin, G.A.

1986-10-10

The /sup 13/C-/sup 13/C spin-spin coupling constants between the carbon nuclei of the vinyl group were measured for a series of vinyl ethers. It was established that the unshared electron pairs of the oxygen atom can make a substantial stereospecific contribution to the direct /sup 13/C-/sup 13/C constants of the adjacent nuclei. The observed effect was used to establish the conformational structure of the compounds.

Superradiators created atom by atom

Science.gov (United States)

Meschede, Dieter

2018-02-01

High radiation rates are usually associated with macroscopic lasers. Laser radiation is “coherent”—its amplitude and phase are well-defined—but its generation requires energy inputs to overcome loss. Excited atoms spontaneously emit in a random and incoherent fashion, and for N such atoms, the emission rate simply increases as N. However, if these atoms are in close proximity and coherently coupled by a radiation field, this microscopic ensemble acts as a single emitter whose emission rate increases as N2 and becomes “superradiant,” to use Dicke's terminology (1). On page 662 of this issue, Kim et al. (2) show the buildup of coherent light fields through collective emission from atomic radiators injected one by one into a resonator field. There is only one atom ever in the cavity, but the emission is still collective and superradiant. These results suggest another route toward thresholdless lasing.

Performance assessment of a new laser system for efficient spin exchange optical pumping in a spin maser measurement of 129Xe EDM

International Nuclear Information System (INIS)

Funayama, C.; Furukawa, T.; Sato, T.; Ichikawa, Y.; Ohtomo, Y.; Sakamoto, Y.; Kojima, S.; Suzuki, T.; Hirao, C.; Chikamori, M.; Hikota, E.; Tsuchiya, M.; Yoshimi, A.; Bidinosti, C. P.; Ino, T.; Ueno, H.; Matsuo, Y.; Fukuyama, T.; Asahi, K.

2015-01-01

We demonstrate spin-exchange optical pumping of 129 Xe atoms with our newly made laser system. The new laser system was prepared to provide higher laser power required for the stable operation of spin maser oscillations in the 129 Xe EDM experiment. We studied the optimum cell temperature and pumping laser power to improve the degree of 129 Xe spin polarization. The best performance was achieved at the cell temperature of 100 ∘ C with the presently available laser power of 1 W. The results show that a more intense laser is required for further improvement of the spin polarization at higher cell temperatures in our experiment

Towards Long-Distance Atom-Photon Entanglement

International Nuclear Information System (INIS)

Rosenfeld, W.; Hocke, F.; Henkel, F.; Krug, M.; Volz, J.; Weber, M.; Weinfurter, H.

2008-01-01

We report the observation of entanglement between a single trapped atom and a single photon at remote locations. The degree of coherence of the entangled atom-photon pair is verified via appropriate local correlation measurements, after communicating the photon via an optical fiber link of 300 m length to a receiver 3.5 m apart. In addition, we measured the temporal evolution of the atomic density matrix after projecting the atom via a state measurement of the photon onto several well-defined spin states. We find that the state of the single atom dephases on a time scale of 150 μs, which represents an important step towards long-distance quantum networking with individual neutral atoms

Experiments with cold hydrogen atoms

International Nuclear Information System (INIS)

Leonas, V.B.

1981-01-01

Numerous investigations of atomic processes in Waseous phase on the surface with participation of ''cold'' hydrogen atoms, made during the last years, are considered. The term ''cold atom'' means the range of relative collision energies E<10 MeV (respectively 'ultracold ' atoms at E< or approximately 1 MeV) which corresponds to the range of temperatures in tens (units) of K degrees. Three main ranges of investigations where extensive experimental programs are realized are considered: study of collisional processes with hydrogen atom participation, hydrogen atoms being of astrophysical interest; study of elastic atom-molecular scattering at superlow energies and studies on the problem of condensed hydrogen. Hydrogen atoms production is realized at dissociation in non-electrode high-frequency or superhigh-frequency discharge. A method of hydrogen quantum generator and of its modifications appeared to be rather an effective means to study collisional changes of spin state of hydrogen atoms. First important results on storage and stabilization of the gas of polarized hydrogen atoms are received

Spin-1 Dirac-Weyl fermions protected by bipartite symmetry

Energy Technology Data Exchange (ETDEWEB)

Lin, Zeren [College of Chemistry and Molecular Engineering, Peking University, Beijing 100871 (China); School of Physics, Peking University, Beijing 100871 (China); Liu, Zhirong, E-mail: LiuZhiRong@pku.edu.cn [College of Chemistry and Molecular Engineering, Peking University, Beijing 100871 (China); Center for Nanochemistry, Beijing National Laboratory for Molecular Sciences (BNLMS), Peking University, Beijing 100871 (China)

2015-12-07

We propose that bipartite symmetry allows spin-1 Dirac-Weyl points, a generalization of the spin-1/2 Dirac points in graphene, to appear as topologically protected at the Fermi level. In this spirit, we provide methodology to construct spin-1 Dirac-Weyl points of this kind in a given 2D space group and get the classification of the known spin-1 systems in the literature. We also apply the workflow to predict two new systems, P3m1-9 and P31m-15, to possess spin-1 at K/K′ in the Brillouin zone of hexagonal lattice. Their stability under various strains is investigated and compared with that of T{sub 3}, an extensively studied model of ultracold atoms trapped in optical lattice with spin-1 also at K/K′.

Atomic-resolution structure of the CAP-Gly domain of dynactin on polymeric microtubules determined by magic angle spinning NMR spectroscopy.

Science.gov (United States)

Yan, Si; Guo, Changmiao; Hou, Guangjin; Zhang, Huilan; Lu, Xingyu; Williams, John Charles; Polenova, Tatyana

2015-11-24

Microtubules and their associated proteins perform a broad array of essential physiological functions, including mitosis, polarization and differentiation, cell migration, and vesicle and organelle transport. As such, they have been extensively studied at multiple levels of resolution (e.g., from structural biology to cell biology). Despite these efforts, there remain significant gaps in our knowledge concerning how microtubule-binding proteins bind to microtubules, how dynamics connect different conformational states, and how these interactions and dynamics affect cellular processes. Structures of microtubule-associated proteins assembled on polymeric microtubules are not known at atomic resolution. Here, we report a structure of the cytoskeleton-associated protein glycine-rich (CAP-Gly) domain of dynactin motor on polymeric microtubules, solved by magic angle spinning NMR spectroscopy. We present the intermolecular interface of CAP-Gly with microtubules, derived by recording direct dipolar contacts between CAP-Gly and tubulin using double rotational echo double resonance (dREDOR)-filtered experiments. Our results indicate that the structure adopted by CAP-Gly varies, particularly around its loop regions, permitting its interaction with multiple binding partners and with the microtubules. To our knowledge, this study reports the first atomic-resolution structure of a microtubule-associated protein on polymeric microtubules. Our approach lays the foundation for atomic-resolution structural analysis of other microtubule-associated motors.

Structure stability and magnetism in graphene impurity complexes with embedded V and Nb atoms

Energy Technology Data Exchange (ETDEWEB)

Thakur, Jyoti [Department of Physics, University College, Kurukshetra University, Kurukshetra 136119, Haryana (India); Kashyap, Manish K., E-mail: manishdft@gmail.com [Department of Physics, Kurukshetra University, Kurukshetra 136119, Haryana (India); Ames Laboratory, U.S. Department of Energy, Iowa State University, Ames, IA 50011-3020 (United States); Taya, Ankur; Rani, Priti [Department of Physics, Kurukshetra University, Kurukshetra 136119, Haryana (India); Saini, Hardev S. [Department of Physics, Guru Jambheshwar University of Science & Technology, Hisar 125001, Haryana (India); Reshak, A.H. [New Technologies – Research Centre, University of West Bohemia, Univerzitni 8, 306 14 Pilsen (Czech Republic); School of Material Engineering, University Malaysia Perlis, 01007 Kangar, Perlis (Malaysia)

2017-07-01

Highlights: • V/Nb embedding in graphene containing monovacancies/divacancies is presented. • Spin polarization near/equal to 100% ensures use of studied nanosystems in spin filter devices. • Bandstructures are analyzed to identify shifting of Dirac cone of graphene. - Abstract: The appearance of vacancy defects could produce appropriate magnetic moment in graphene and the sensitivity to absorb atoms/molecules also increases with this. In this direction, a DFT study of embedding V and Nb atom in graphene containing monovacancies (MV) and divacancies (DV) is reported. Complete/almost complete spin polarization is detected for V/Nb embedding. The origin of magnetism has been identified via interaction of 3d-states of embedded atom with C-p states present in the vicinity of embedded site. The band structures have been analyzed to counter the observed semiconducting nature of graphene in minority spin on embedding V/Nb atom. The isosurface analysis also confirms the induced magnetism of present nanosystems. The present results reveal that these nanosystems have the potential for futuristic applications like spintronics and energy resources.

Superexchange-mediated magnetization dynamics with ultracold alkaline-earth atoms in an optical lattice

International Nuclear Information System (INIS)

Zhu Shaobing; Qian Jun; Wang Yuzhu

2017-01-01

Superexchange and inter-orbital spin-exchange interactions are key ingredients for understanding (orbital) quantum magnetism in strongly correlated systems and have been realized in ultracold atomic gases. Here we study the spin dynamics of ultracold alkaline-earth atoms in an optical lattice when the two exchange interactions coexist. In the superexchange interaction dominating regime, we find that the time-resolved spin imbalance shows a remarkable modulated oscillation, which can be attributed to the interplay between local and nonlocal quantum mechanical exchange mechanisms. Moreover, the filling of the long-lived excited atoms affects the collapse and revival of the magnetization dynamics. These observations can be realized in state-dependent optical lattices combined with the state-of-the-art advances in optical lattice clock spectroscopy. (paper)

Many-body dynamics of holes in a driven, dissipative spin chain of Rydberg superatoms

Science.gov (United States)

Letscher, Fabian; Petrosyan, David; Fleischhauer, Michael

2017-11-01

Strong, long-range interactions between atoms in high-lying Rydberg states can suppress multiple Rydberg excitations within a micron-sized trapping volume and yield sizable Rydberg level shifts at larger distances. Ensembles of atoms in optical microtraps then form Rydberg superatoms with collectively enhanced transition rates to the singly excited state. These superatoms can represent mesoscopic, strongly interacting spins. We study a regular array of such effective spins driven by a laser field tuned to compensate the interaction-induced level shifts between neighboring superatoms. During the initial transient, a few excited superatoms seed a cascade of resonantly facilitated excitation of large clusters of superatoms. Due to spontaneous decay, the system then relaxes to the steady state having nearly universal Rydberg excitation density {ρ }{{R}}=2/3. This state is characterized by highly non-trivial equilibrium dynamics of quasi-particles—excitation holes in the lattice of Rydberg excited superatoms. We derive an effective many-body model that accounts for hole mobility as well as continuous creation and annihilation of holes upon collisions with each other. We find that holes exhibit a nearly incompressible liquid phase with highly sub-Poissonian number statistics and finite-range density-density correlations.

Rb-129Xe spin-exchange rates due to binary and three-body collisions at high Xe pressures

International Nuclear Information System (INIS)

Cates, G.D.; Fitzgerald, R.J.; Barton, A.S.; Bogorad, P.; Gatzke, M.; Newbury, N.R.; Saam, B.

1992-01-01

We have studied the spin relaxation of 129 Xe nuclei due to collisions with Rb atoms at Xe pressures of 245--1817 Torr. Our results can be characterized by two parameters, the Rb- 129 Xe velocity-averaged binary spin-exchange cross section left-angle σv right-angle and a rate γ M that characterizes spin relaxation due to van der Waals molecules. Our results complement earlier studies performed at Xe pressures of about 1 Torr and N 2 pressures of 10--100 Torr. This work is useful for predicting spin-exchange rates between polarized Rb atoms and 129 Xe nuclei

Contactless friction and the {sup 3}He-{sup 4}He dimer. Studies with the atomic-beam spin-echo spectrometer; Kontaktlose Reibung und das {sup 3}He-{sup 4}He-Dimer. Untersuchungen mit dem Atomstrahlspinechospektrometer

Energy Technology Data Exchange (ETDEWEB)

Janke, Matthias

2016-04-20

In this thesis the time of flight resolved atomic beam spin echo method (SEToF) is applied to a {sup 3}He-beam for the first time and studied systematically. This method is shown to be superior to the usual atomic beam spin echo technique. With SEToF it is possible to almost completely remove unpolarized background and to reach a beam polarisation close to 100%. The SEToF technique is shown to be crucial for the first experimental proof of the existence of the {sup 3}He-{sup 4}He dimer. This dimer is the weakest bound van-der-Waals-molecule known to date. Furthermore, a drag force between an atom and a dielectric surface is detected originating from the fluctuating dipole moment of the atom. Not only the measured friction coefficients match their theoretical predictions perfectly, but our data also shows the correct temperature dependence. A great many technological renewals and improvements were installed in the apparatus during this thesis work. They have become necessary or sensible due to the relocation of the physics institute. A few of them are documented and motivated in this thesis.

Inelastic tunneling spectroscopy for magnetic atoms and the Kondo resonance

International Nuclear Information System (INIS)

Goldberg, E C; Flores, F

2013-01-01

The interaction between a single magnetic atom and the metal environment (including a magnetic field) is analyzed by introducing an ionic Hamiltonian combined with an effective crystal-field term, and by using a Green-function equation of motion method. This approach describes the inelastic electron tunneling spectroscopy and the Kondo resonances as due to atomic spin fluctuations associated with electron co-tunneling processes between the leads and the atom. We analyze in the case of Fe on CuN the possible spin fluctuations between states with S = 2 and 3/2 or 5/2 and conclude that the experimentally found asymmetries in the conductance with respect to the applied bias, and its marked structures, are well explained by the 2↔3/2 spin fluctuations. The case of Co is also considered and shown to present, in contrast with Fe, a resonance at the Fermi energy corresponding to a Kondo temperature of 6 K. (paper)

Spin resonance with trapped ions

Energy Technology Data Exchange (ETDEWEB)

Wunderlich, Ch; Balzer, Ch; Hannemann, T; Mintert, F; Neuhauser, W; Reiss, D; Toschek, P E [Institut fuer Laser-Physik, Universitaet Hamburg, Jungiusstrasse 9, 20355 Hamburg (Germany)

2003-03-14

A modified ion trap is described where experiments (in particular related to quantum information processing) that usually require optical radiation can be carried out using microwave or radio frequency electromagnetic fields. Instead of applying the usual methods for coherent manipulation of trapped ions, a string of ions in such a modified trap can be treated like a molecule in nuclear magnetic resonance experiments taking advantage of spin-spin coupling. The collection of trapped ions can be viewed as an N-qubit molecule with adjustable spin-spin coupling constants. Given N identically prepared quantum mechanical two-level systems (qubits), the optimal strategy to estimate their quantum state requires collective measurements. Using the ground state hyperfine levels of electrodynamically trapped {sup 171}Yb{sup +}, we have implemented an adaptive algorithm for state estimation involving sequential measurements on arbitrary qubit states.

Spin resonance with trapped ions

International Nuclear Information System (INIS)

Wunderlich, Ch; Balzer, Ch; Hannemann, T; Mintert, F; Neuhauser, W; Reiss, D; Toschek, P E

2003-01-01

A modified ion trap is described where experiments (in particular related to quantum information processing) that usually require optical radiation can be carried out using microwave or radio frequency electromagnetic fields. Instead of applying the usual methods for coherent manipulation of trapped ions, a string of ions in such a modified trap can be treated like a molecule in nuclear magnetic resonance experiments taking advantage of spin-spin coupling. The collection of trapped ions can be viewed as an N-qubit molecule with adjustable spin-spin coupling constants. Given N identically prepared quantum mechanical two-level systems (qubits), the optimal strategy to estimate their quantum state requires collective measurements. Using the ground state hyperfine levels of electrodynamically trapped 171 Yb + , we have implemented an adaptive algorithm for state estimation involving sequential measurements on arbitrary qubit states

Collection of laws and ordinances concerning regulation of atomic energy, 1991 edition

International Nuclear Information System (INIS)

1990-01-01

This is the collection of the laws and ordinances on the regulation of atomic energy, 1991 edition, published under the supervision of Nuclear Safety Bureau, Science and Technology Agency. First, the abbreviated indication of the laws and ordinances is shown. The contents are those as of September 30, 1990. 12 basic laws and ordinances, 45 laws and ordinances on the regulation of nuclear raw materials, nuclear fuel materials and nuclear reactors, 26 laws and ordinances on the prevention of the radiation injuries due to radioisotopes and others, and 29 related laws and ordinances are collected in this book. (K.I.)

Enhanced Tunnel Spin Injection into Graphene using Chemical Vapor Deposited Hexagonal Boron Nitride

Science.gov (United States)

Kamalakar, M. Venkata; Dankert, André; Bergsten, Johan; Ive, Tommy; Dash, Saroj P.

2014-01-01

The van der Waals heterostructures of two-dimensional (2D) atomic crystals constitute a new paradigm in nanoscience. Hybrid devices of graphene with insulating 2D hexagonal boron nitride (h-BN) have emerged as promising nanoelectronic architectures through demonstrations of ultrahigh electron mobilities and charge-based tunnel transistors. Here, we expand the functional horizon of such 2D materials demonstrating the quantum tunneling of spin polarized electrons through atomic planes of CVD grown h-BN. We report excellent tunneling behavior of h-BN layers together with tunnel spin injection and transport in graphene using ferromagnet/h-BN contacts. Employing h-BN tunnel contacts, we observe enhancements in both spin signal amplitude and lifetime by an order of magnitude. We demonstrate spin transport and precession over micrometer-scale distances with spin lifetime up to 0.46 nanosecond. Our results and complementary magnetoresistance calculations illustrate that CVD h-BN tunnel barrier provides a reliable, reproducible and alternative approach to address the conductivity mismatch problem for spin injection into graphene. PMID:25156685

Optical-coupling nuclear spin maser under highly stabilized low static field

Energy Technology Data Exchange (ETDEWEB)

Yoshimi, A., E-mail: yoshimi@ribf.riken.jp [RIKEN Nishina Center (Japan); Inoue, T.; Uchida, M.; Hatakeyama, N.; Asahi, K. [Tokyo Institute of Technology, Department of Physics (Japan)

2008-01-15

A nuclear spin maser of a new type, that employs a feedback scheme based on optical nuclear spin detection, has been fabricated. The spin maser is operated at a low static field of 30 mG by using the optical detection method. The frequency stability and precision of the spin maser have been improved by a highly stabilized current source for the static magnetic field. An experimental setup to search for an electric dipole moment (EDM) in {sup 129}Xe atom is being developed.

Quantum Computing with an Electron Spin Ensemble

DEFF Research Database (Denmark)

Wesenberg, Janus; Ardavan, A.; Briggs, G.A.D.

2009-01-01

We propose to encode a register of quantum bits in different collective electron spin wave excitations in a solid medium. Coupling to spins is enabled by locating them in the vicinity of a superconducting transmission line cavity, and making use of their strong collective coupling to the quantized...

Magnetoresistance through spin-polarized p states

International Nuclear Information System (INIS)

Papanikolaou, Nikos

2003-01-01

We present a theoretical study of the ballistic magnetoresistance in Ni contacts using first-principles, atomistic, electronic structure calculations. In particular we investigate the role of defects in the contact region with the aim of explaining the recently observed spectacular magnetoresistance ratio. Our results predict that the possible presence of spin-polarized oxygen in the contact region could explain conductance changes by an order of magnitude. Electronic transport essentially occurs through spin-polarized oxygen p states, and this mechanism gives a much higher magnetoresistance than that obtained assuming clean atomically sharp domain walls alone

Angular momentum effects in electron scattering from atoms

International Nuclear Information System (INIS)

Williams, J F; Cvejanovie, D; Samarin, S; Pravica, L; Napier, S; Sergeant, A

2007-01-01

This paper concerns angular momentum-dependent phenomena in excited gas-phase atoms using incident photons or electrons in scattering experiments. A brief overview indicates the main capabilities of experimental techniques and the information which can be deduced about atomic structure and dynamics from conservation of momenta with measurement of polarization and detection of the number of emerging electrons, photons and ions. Maximum information may be obtained when the incident particles and the targets are state-selected both before and after scattering. The fundamental scattering amplitudes and their relative phases, and consequently derived quantities such as the parameters describing the electron charge cloud of the atomic target, have enabled significant advances of understanding of collision mechanisms. The angular momentum-dependent scattering probabilities change when, for example, the spin-orbit interaction for the target electrons becomes large compared with the Coulomb electron-electron interactions and also when electron exchange and the relative orientation of the electron spins change. Several examples are discussed to indicate significant principles and recent advances. Major contributions to this field from the technology associated with electron spin production and detection time, as well as time-coincidence detection, are discussed. New results from the authors' laboratory are presented

A Spin-Flip Cavity for Microwave Spectroscopy of Antihydrogen

CERN Document Server

Federmann, Silke; Widmann, Eberhard

The present thesis is a contribution to the Asacusa (Atomic Spectroscopy And Collisions Using Slow Antiprotons) experiment. The aim of this experiment is to measure the ground-state hyperfine structure of antihydrogen. This is done using a Rabi-like spectrometer line consisting of an antihydrogen source, a microwave cavity, a sextupole magnet and a detector. The cavity induces spin-flip transitions in the ground-state hyperfine levels of antihydrogen whereas the sextupole magnet selects the antihydrogen atoms according to their spin state. Such a configuration allows the measurements of the hyperfine transition in antihydrogen with very high precision. A comparison with the corresponding transitions in hydrogen would thus provide a very sensitive test of the charge-parity-time (Cpt) symmetry. In the context of this thesis, the central piece of this spectrometer line, the spin flip cavity, was designed and implemented. The delicacy of this task was achieving the required field homogeneity: It needs to be bette...

Towards Quantum Simulation with Circular Rydberg Atoms

Directory of Open Access Journals (Sweden)

T. L. Nguyen

2018-02-01

Full Text Available The main objective of quantum simulation is an in-depth understanding of many-body physics, which is important for fundamental issues (quantum phase transitions, transport, … and for the development of innovative materials. Analytic approaches to many-body systems are limited, and the huge size of their Hilbert space makes numerical simulations on classical computers intractable. A quantum simulator avoids these limitations by transcribing the system of interest into another, with the same dynamics but with interaction parameters under control and with experimental access to all relevant observables. Quantum simulation of spin systems is being explored with trapped ions, neutral atoms, and superconducting devices. We propose here a new paradigm for quantum simulation of spin-1/2 arrays, providing unprecedented flexibility and allowing one to explore domains beyond the reach of other platforms. It is based on laser-trapped circular Rydberg atoms. Their long intrinsic lifetimes, combined with the inhibition of their microwave spontaneous emission and their low sensitivity to collisions and photoionization, make trapping lifetimes in the minute range realistic with state-of-the-art techniques. Ultracold defect-free circular atom chains can be prepared by a variant of the evaporative cooling method. This method also leads to the detection of arbitrary spin observables with single-site resolution. The proposed simulator realizes an XXZ spin-1/2 Hamiltonian with nearest-neighbor couplings ranging from a few to tens of kilohertz. All the model parameters can be dynamically tuned at will, making a large range of simulations accessible. The system evolution can be followed over times in the range of seconds, long enough to be relevant for ground-state adiabatic preparation and for the study of thermalization, disorder, or Floquet time crystals. The proposed platform already presents unrivaled features for quantum simulation of regular spin chains. We

Towards Quantum Simulation with Circular Rydberg Atoms

Science.gov (United States)

Nguyen, T. L.; Raimond, J. M.; Sayrin, C.; Cortiñas, R.; Cantat-Moltrecht, T.; Assemat, F.; Dotsenko, I.; Gleyzes, S.; Haroche, S.; Roux, G.; Jolicoeur, Th.; Brune, M.

2018-01-01

The main objective of quantum simulation is an in-depth understanding of many-body physics, which is important for fundamental issues (quantum phase transitions, transport, …) and for the development of innovative materials. Analytic approaches to many-body systems are limited, and the huge size of their Hilbert space makes numerical simulations on classical computers intractable. A quantum simulator avoids these limitations by transcribing the system of interest into another, with the same dynamics but with interaction parameters under control and with experimental access to all relevant observables. Quantum simulation of spin systems is being explored with trapped ions, neutral atoms, and superconducting devices. We propose here a new paradigm for quantum simulation of spin-1 /2 arrays, providing unprecedented flexibility and allowing one to explore domains beyond the reach of other platforms. It is based on laser-trapped circular Rydberg atoms. Their long intrinsic lifetimes, combined with the inhibition of their microwave spontaneous emission and their low sensitivity to collisions and photoionization, make trapping lifetimes in the minute range realistic with state-of-the-art techniques. Ultracold defect-free circular atom chains can be prepared by a variant of the evaporative cooling method. This method also leads to the detection of arbitrary spin observables with single-site resolution. The proposed simulator realizes an X X Z spin-1 /2 Hamiltonian with nearest-neighbor couplings ranging from a few to tens of kilohertz. All the model parameters can be dynamically tuned at will, making a large range of simulations accessible. The system evolution can be followed over times in the range of seconds, long enough to be relevant for ground-state adiabatic preparation and for the study of thermalization, disorder, or Floquet time crystals. The proposed platform already presents unrivaled features for quantum simulation of regular spin chains. We discuss

Chip-Scale Combinatorial Atomic Navigator (C-SCAN) Low Drift Nuclear Spin Gyroscope

Science.gov (United States)

2018-01-01

suggestions for reducing this burden, to Department of Defense, Washington Headquarters Services, Directorate for Information Operations and Reports (0704...spin-exchange relaxation in a finite magnetic field. We operated the gyroscope using a Ramsey-type interrogation sequence with nuclear spin precession...shift by a factor of 105. Here we use the approach of a Ramsey clock interrogation scheme, where the optical pumping, free evolution, and measurement

Collectivity of high spin states in {sup 84}Zr

Energy Technology Data Exchange (ETDEWEB)

Lister, C.J.; Blumenthal, D.; Crowell, B. [and others

1995-08-01

{sup 84}Zr is one of the most extensively studied of the A {approximately} 80 rotors, both from theoretical and experimental approaches. It was predicted to be a good candidate to support superdeformation, and to show interesting spectroscopic properties including saturation of its shell-model space at lower spin. We performed an experiment using Gammasphere in its early implementation phase. The reaction of {sup 29}Si on {sup 58}Ni was used to strongly populate {sup 84}Zr at high spin. Thin and thick targets were used to allow the extraction of transitional matrix elements at very high spin, and to allow a sensitive search for superdeformed states. Data analysis is in progress. The large data set allowed us to extend the previously known bands considerably. Candidates for a staggered M1-band, found previously {sup 86}Zr, were located. To date, no evidence for superdeformed bands was found. Analysis was slowed by the relocation of all the participants in this experiment, but we hope to complete the lifetime analysis this year. This analysis has become especially topical, due to reported measurements of superdeformation in this region.

Lateral spin injection and detection via electrodeposited Fe/GaAs contacts

OpenAIRE

Majumder, Sarmita

2013-01-01

Experimental studies of lateral spin injection and detection through electrodeposited Fe/GaAs tunnel contacts are reported in this thesis. An enhanced spin valve voltage is demonstrated via non-local lateral spin transport measurements compared to their vacuum-deposited counterparts. We have proposed a simple theoretical model to explain this result. Combined with experimental evidence for interfacial oxygen from atom probe tomography, we speculate that the enhancements occur due to a magne...

Electron spin resonance of spin-trapped radicals of amines and polyamines

International Nuclear Information System (INIS)

Mossoba, M.M.; Rosenthal, Ionel; Riesz, Peter

1982-01-01

The reactions of hydroxyl radicals with methylamine, dimethylamine, trimethylamine, diethylamine, sec-butylamine, ethylene-diamine, 1,3-diaminopropane, putrescine, cadaverine, 1,7-diaminoheptane, ornithine, spermidine, spermine, agmatine, and arcaine in aqueous solutions have been investigated by spin-trapping and esr. Hydroxyl radicals were generated by the uv photolysis of H 2 O 2 and 2-methyl-2-nitrosopropane (MNP) was used as the spin-trap. The effects of ionizing radiation on the same polyamines in the polycrystalline state were also investigated. The free radicals produced by ν-radiolysis of these solids at room temperature in the absence of air were identified by dissolution in aqueous solutions of MNP. The predominant reaction of OH radicals with amines and polyamines below pH 7 was the abstraction of hydrogen atoms from a carbon that is not adjacent to the protonated amino group. For agmatine and arcaine which contain guanidinium groups abstraction occurred from the α-CH. Dimethylamine was oxidized to the dimethylnitroxyl radical by H 2 O 2 in the dark. ν-Radiolysis of polyamines in the polycrystalline state generated radicals due to H-abstraction from either the α-Ch or from a carbon atom in the middle of the alkyl chain. The deamination radical was obtained from ornithine

Scattering resonances in a low-dimensional Rashba-Dresselhaus spin-orbit coupled quantum gas

Science.gov (United States)

Wang, Su-Ju; Blume, D.

2017-04-01

Confinement-induced resonances allow for the tuning of the effective one-dimensional coupling constant. When the scattering state associated with the ground transverse mode is brought into resonance with the bound state attached to the energetically excited transverse modes, the atoms interact through an infinitely strong repulsion. This provides a route to realize the Tonks-Girardeau gas. On the other hand, the realization of synthetic gauge fields in cold atomic systems has attracted a lot of attention. For instance, bound-state formation is found to be significantly modified in the presence of spin-orbit coupling in three dimensions. This motivates us to study ultracold collisions between two Rashba-Dresselhaus spin-orbit coupled atoms in a quasi-one-dimensional geometry. We develop a multi-channel scattering formalism that accounts for the external transverse confinement and the spin-orbit coupling terms. The interplay between these two single-particle terms is shown to give rise to new scattering resonances. In particular, it is analyzed what happens when the scattering energy crosses the various scattering thresholds that arise from the single-particle confinement and the spin-orbit coupling. Support by the NSF is gratefully acknowledged.

Restricted magnetically balanced basis applied for relativistic calculations of indirect nuclear spin-spin coupling tensors in the matrix Dirac-Kohn-Sham framework

International Nuclear Information System (INIS)

Repisky, Michal; Komorovsky, Stanislav; Malkina, Olga L.; Malkin, Vladimir G.

2009-01-01

The relativistic four-component density functional approach based on the use of restricted magnetically balanced basis (mDKS-RMB), applied recently for calculations of NMR shielding, was extended for calculations of NMR indirect nuclear spin-spin coupling constants. The unperturbed equations are solved with the use of a restricted kinetically balanced basis set for the small component while to solve the second-order coupled perturbed DKS equations a restricted magnetically balanced basis set for the small component was applied. Benchmark relativistic calculations have been carried out for the X-H and H-H spin-spin coupling constants in the XH 4 series (X = C, Si, Ge, Sn and Pb). The method provides an attractive alternative to existing approximate two-component methods with transformed Hamiltonians for relativistic calculations of spin-spin coupling constants of heavy-atom systems. In particular, no picture-change effects arise in our method for property calculations

Spin-Wave Diode

Directory of Open Access Journals (Sweden)

Jin Lan (兰金

2015-12-01

Full Text Available A diode, a device allowing unidirectional signal transmission, is a fundamental element of logic structures, and it lies at the heart of modern information systems. The spin wave or magnon, representing a collective quasiparticle excitation of the magnetic order in magnetic materials, is a promising candidate for an information carrier for the next-generation energy-saving technologies. Here, we propose a scalable and reprogrammable pure spin-wave logic hardware architecture using domain walls and surface anisotropy stripes as waveguides on a single magnetic wafer. We demonstrate theoretically the design principle of the simplest logic component, a spin-wave diode, utilizing the chiral bound states in a magnetic domain wall with a Dzyaloshinskii-Moriya interaction, and confirm its performance through micromagnetic simulations. Our findings open a new vista for realizing different types of pure spin-wave logic components and finally achieving an energy-efficient and hardware-reprogrammable spin-wave computer.

Muon spin relaxation in ferromagnets. Pt. 1

International Nuclear Information System (INIS)

Lovesey, S.W.; Karlsson, E.B.

1991-04-01

Expressions for the dipolar and hyperfine contributions to the relaxation rate of muons implanted in a ferromagnet are presented and analysed using the Heisenberg model of spin-waves including dipolar and Zeeman energies. Calculations for EuO indicate that relaxation is likely to be dominated by the hyperfine mechanism, even if the ratio of the hyperfine and dipolar coupling constants is small. The hyperfine mechanism is sensitive to the dipolar energy of the atomic spins, whereas the dipolar mechanisms depend essentially on the exchange energy. For both mechanisms there is an almost quadratic dependence on temperature, throughout much of the ordered magnetic phase, which reflects two-spin-wave difference events from the Raman-type relaxation processes. (author)

Electromagnetic transitions in the atom

International Nuclear Information System (INIS)

Ulehla, I.; Suk, M.; Trka, Z.

1990-01-01

Methods to achieve excitation of atoms are outlined and conditions necessary for the occurrence of electromagnetic transitions in the atomic shell are given. Radiative transitions between the energy states of the atom include stimulated absorption, spontaneous emission, and stimulated emission. Selection rules applying to the majority of observed transitions are given. The parity concept is explained. It is shown how the electromagnetic field and its interaction with the magnetic moment of the atom lead to a disturbance of the energy states of the atom and the occurrence of various electro-optical and magneto-optical phenomena. The Stark effect and electron spin resonance are described. X-rays and X-ray spectra, the Auger effect and the internal photoeffect are also dealt with. The principle of the laser is explained. (M.D.). 22 figs., 1 tab

Spin Hall effects

Science.gov (United States)

Sinova, Jairo; Valenzuela, Sergio O.; Wunderlich, J.; Back, C. H.; Jungwirth, T.

2015-10-01

Spin Hall effects are a collection of relativistic spin-orbit coupling phenomena in which electrical currents can generate transverse spin currents and vice versa. Despite being observed only a decade ago, these effects are already ubiquitous within spintronics, as standard spin-current generators and detectors. Here the theoretical and experimental results that have established this subfield of spintronics are reviewed. The focus is on the results that have converged to give us the current understanding of the phenomena, which has evolved from a qualitative to a more quantitative measurement of spin currents and their associated spin accumulation. Within the experimental framework, optical-, transport-, and magnetization-dynamics-based measurements are reviewed and linked to both phenomenological and microscopic theories of the effect. Within the theoretical framework, the basic mechanisms in both the extrinsic and intrinsic regimes are reviewed, which are linked to the mechanisms present in their closely related phenomenon in ferromagnets, the anomalous Hall effect. Also reviewed is the connection to the phenomenological treatment based on spin-diffusion equations applicable to certain regimes, as well as the spin-pumping theory of spin generation used in many measurements of the spin Hall angle. A further connection to the spin-current-generating spin Hall effect to the inverse spin galvanic effect is given, in which an electrical current induces a nonequilibrium spin polarization. This effect often accompanies the spin Hall effect since they share common microscopic origins. Both can exhibit the same symmetries when present in structures comprising ferromagnetic and nonmagnetic layers through their induced current-driven spin torques or induced voltages. Although a short chronological overview of the evolution of the spin Hall effect field and the resolution of some early controversies is given, the main body of this review is structured from a pedagogical

Optical pumping production of spin polarized hydrogen

International Nuclear Information System (INIS)

Knize, R.J.; Happer, W.; Cecchi, J.L.

1984-01-01

There has been much interest recently in the production of large quantities of spin polarized hydrogen in various fields including controlled fusion, quantum fluids, high energy, and nuclear physics. One promising method for the development of large quantities of spin polarized hydrogen is the utilization of optical pumping with a laser. Optical pumping is a process where photon angular momentum is converted into electron and nuclear spin. The advent of tunable CW dye lasers (approx. 1 watt) allow the production of greater than 10 18 polarized atoms/sec. We have begun a program at Princeton to investigate the physics and technology of using optical pumping to produce large quantities of spin polarized hydrogen. Initial experiments have been done in small closed glass cells. Eventually, a flowing system, open target, or polarized ion source could be constructed

Harmonic detection of magnetic resonance for sensitivity improvement of optical atomic magnetometers

Energy Technology Data Exchange (ETDEWEB)

Ranjbaran, M. [Laser and Plasma Research Institute, Shahid Beheshti University, Tehran (Iran, Islamic Republic of); Tehranchi, M.M., E-mail: teranchi@sbu.ac.ir [Laser and Plasma Research Institute, Shahid Beheshti University, Tehran (Iran, Islamic Republic of); Physics Department, Shahid Beheshti University, Tehran (Iran, Islamic Republic of); Hamidi, S.M. [Laser and Plasma Research Institute, Shahid Beheshti University, Tehran (Iran, Islamic Republic of); Khalkhali, S.M.H. [Physics Department, Kharazmi University, Tehran (Iran, Islamic Republic of)

2017-02-15

Highly sensitive atomic magnetometers use optically detected magnetic resonance of atomic spins to measure extremely weak magnetic field changes. The magnetometer sensitivity is directly proportional to the ratio of intensity to line-shape of the resonance signal. To obtain narrower resonance signal, we implemented harmonic detection of magnetic resonance method in M{sub x} configuration. The nonlinear spin polarization dynamics in detection of the higher harmonics were employed in phenomenological Bloch equations. The measured and simulated harmonic components of the resonance signals in frequency domain yielded significantly narrower line-width accompanying much improved sensitivity. Our results confirm the sensitivity improvement by a factor of two in optical atomic magnetometer via second harmonic signal which can open a new insight in the weak magnetic field measurement system design. - Highlights: • Highly sensitive atomic magnetometers have been used to measure weak magentic filed. • To obtain narrower resonance signal, we impalnted harmonic detection of magnetic resonance. • The nonlinear spin polarization dynamics in detetion of the higher harmonics were imployed.

Excitation of bond-alternating spin-1/2 Heisenberg chains by tunnelling electrons

International Nuclear Information System (INIS)

Gauyacq, J-P; Lorente, N

2014-01-01

Inelastic electron tunneling spectra (IETS) are evaluated for spin-1/2 Heisenberg chains showing different phases of their spin ordering. The spin ordering is controlled by the value of the two different Heisenberg couplings on the two sides of each of the chain's atoms (bond-alternating chains). The perfect anti-ferromagnetic phase, i.e. a unique exchange coupling, marks a topological quantum phase transition (TQPT) of the bond-alternating chain. Our calculations show that the TQPT is recognizable in the excited states of the chain and hence that IETS is in principle capable of discriminating the phases. We show that perfectly symmetric chains, such as closed rings mimicking infinite chains, yield the same spectra on both sides of the TQPT and IETS cannot reveal the nature of the spin phase. However, for finite size open chains, both sides of the TQPT are associated with different IETS spectra, especially on the edge atoms, thus outlining the transition. (paper)

Quantum information entropies of ultracold atomic gases in a ...

Indian Academy of Sciences (India)

The position and momentum space information entropies of weakly interacting trapped atomic Bose–Einstein condensates and spin-polarized trapped atomic Fermi gases at absolute zero temperature are evaluated. We find that sum of the position and momentum space information entropies of these quantum systems ...

Spin Transport in Semiconductor heterostructures

International Nuclear Information System (INIS)

Marinescu, Domnita Catalina

2011-01-01

The focus of the research performed under this grant has been the investigation of spin transport in magnetic semiconductor heterostructures. The interest in these systems is motivated both by their intriguing physical properties, as the physical embodiment of a spin-polarized Fermi liquid, as well as by their potential applications as spintronics devices. In our work we have analyzed several different problems that affect the spin dynamics in single and bi-layer spin-polarized two-dimensional (2D) systems. The topics of interests ranged from the fundamental aspects of the electron-electron interactions, to collective spin and charge density excitations and spin transport in the presence of the spin-orbit coupling. The common denominator of these subjects is the impact at the macroscopic scale of the spin-dependent electron-electron interaction, which plays a much more subtle role than in unpolarized electron systems. Our calculations of several measurable parameters, such as the excitation frequencies of magneto-plasma modes, the spin mass, and the spin transresistivity, propose realistic theoretical estimates of the opposite-spin many-body effects, in particular opposite-spin correlations, that can be directly connected with experimental measurements.

Abrupt relaxation in high-spin molecules

International Nuclear Information System (INIS)

Chang, C.-R.; Cheng, T.C.

2000-01-01

Mean-field model suggests that the rate of resonant quantum tunneling in high-spin molecules is not only field-dependent but also time-dependent. The relaxation-assisted resonant tunneling in high-spin molecules produces an abrupt magnetization change during relaxation. When the applied field is very close to the resonant field, a time-dependent interaction field gradually shifts the energies of different collective spin states, and magnetization tunneling is observed as two energies of the spin states coincide

The single-ion anisotropy effects in the mixed-spin ternary-alloy

Science.gov (United States)

Albayrak, Erhan

2018-04-01

The effect of single-ion anisotropy on the thermal properties of the ternary-alloy in the form of ABpC1-p is investigated on the Bethe lattice (BL) in terms of exact recursion relations. The simulation on the BL consists of placing A atoms (spin-1/2) on the odd shells and randomly placing B (spin-3/2) or C (spin-5/2) atoms with concentrations p and 1 - p, respectively, on the even shells. The phase diagrams are calculated in possible planes spanned by the system parameters: temperature, single-ion anisotropy, concentration and ratio of the bilinear interaction parameters for z = 3 corresponding to the honeycomb lattice. It is found that the crystal field drives the system to the lowest possible state therefore reducing the temperatures of the critical lines in agreement with the literature.

Measuring Pancharatnam's relative phase for SO(3) evolutions using spin polarimetry

International Nuclear Information System (INIS)

Larsson, Peter; Sjoeqvist, Erik

2003-01-01

In polarimetry, a superposition of internal quantal states is exposed to a single Hamiltonian and information about the evolution of the quantal states is inferred from projection measurements on the final superposition. In this framework, we here extend the polarimetric test of Pancharatnam's relative phase for spin-(1/2) proposed by Wagh and Rakhecha [Phys. Lett. A 197, 112 (1995)] to spin j≥1 undergoing noncyclic SO(3) evolution. We demonstrate that the output intensity for higher spin values is a polynomial function of the corresponding spin-(1/2) intensity. We further propose a general method to extract the noncyclic SO(3) phase and visibility by rigid translation of two π/2 spin flippers. Polarimetry on higher spin states may in practice be done with spin polarized atomic beams

Energy levels of a spin-orbit-coupled Bose-Einstein condensate in a double-well potential

Science.gov (United States)

Wang, Wen-Yuan; Cao, Hui; Zhu, Shi-Liang; Liu, Jie; Fu, Li-Bin

2015-02-01

We investigate the energy levels of a spin-orbit-coupled Bose-Einstein condensate in a double-well potential under the mean-field approximation. We find that the energy levels of the system can be significantly influenced by the atomic interactions. Without atomic interaction, four energy levels change linearly with the tunneling amplitude, the Raman coupling, and the spin-orbit coupling. However, whenever atomic interaction is considered, three more energy levels will appear, which have a nonlinear dependence on those parameters above. These three energy levels are multi-degenerate and related to the macro-symmetry of the system.

Electron spin-lattice relaxation mechanisms of radiation produced trapped electrons and hydrogen atoms in aqueous and organic glassy matrices. Modulation of electron nuclear dipolar interaction by tunnelling modes in a glassy matrix. [. gamma. rays

Energy Technology Data Exchange (ETDEWEB)

Bowman, M K; Kevan, L [Wayne State Univ., Detroit, Mich. (USA). Dept. of Chemistry

1977-01-01

The spin lattice relaxation of trapped electrons in aqueous and organic glasses and trapped hydrogen atoms in phosphoric acid glass has been directly studied as a function of temperature by the saturation recovery method. Below 50 to 100 K, the major spin lattice relaxation mechanism involves modulation of the electron nuclear dipolar (END) interaction with nuclei in the radical's environment by tunnelling of those nuclei between two or more positions. This relaxation mechanism occurs with high efficiency and has a characteristic linear temperature dependence. The tunnelling nuclei around trapped electrons do not seem to involve the nearest neighbor nuclei which are oriented by the electron in the process of solvation. Instead the tunnelling nuclei typically appear to be next nearest neighbors to the trapped electron. The identities of the tunnelling nuclei have been deduced by isotopic substitution and are attributed to: Na in 10 mol dm/sup -3/ NaOH aqueous glass, ethyl protons in ethanol glass, methyl protons in methanol glass and methyl protons in MTHF glass. For trapped hydrogen atoms in phosphoric acid, the phosphorus nuclei appear to be the effective tunnelling nuclei. Below approximately 10 K the spin lattice relaxation is dominated by a temperature independent cross relaxation term for H atoms in phosphoric acid glass and for electrons in 10 mol dm/sup -3/ NaOH aqueous glass, but not for electrons in organic glasses. This is compared with recent electron-electron double resonance studies of cross relaxation in these glasses. The spin lattice relaxation of O/sup -/ formed in 10 mol dm/sup -3/ NaOH aqueous glass was also studied and found to be mainly dominated by a Raman process with an effective Debye temperature of about 100 K.

2,6-di-tert-butylphenylvinyl ether: effect of the unshared oxygen electron pair on the /sup 13/C-/sup 13/C spin-spin interaction constant

Energy Technology Data Exchange (ETDEWEB)

Krivdin, L.B.; Shcherbakov, V.V.; Glukhikh, N.G.; Sigalov, V.M.; Kalabin, G.A.

1987-07-10

Vinyl ethers were prepared by the well-known Favorskii-Shostakovskii method. The purity of the compounds was controlled by GLC and by the PMR and /sup 13/C NMR spectra. The proximity of sp/sup 7/-hybridized unshared pair of oxygen atoms result in a secondary, positive contribution in the constant of spin-spin interaction between neighboring carbon nuclei in the aromatic ring.

Semiclassical treatment of transport and spin relaxation in spin-orbit coupled systems

Energy Technology Data Exchange (ETDEWEB)

Lueffe, Matthias Clemens

2012-02-10

The coupling of orbital motion and spin, as derived from the relativistic Dirac equation, plays an important role not only in the atomic spectra but as well in solid state physics. Spin-orbit interactions are fundamental for the young research field of semiconductor spintronics, which is inspired by the idea to use the electron's spin instead of its charge for fast and power saving information processing in the future. However, on the route towards a functional spin transistor there is still some groundwork to be done, e.g., concerning the detailed understanding of spin relaxation in semiconductors. The first part of the present thesis can be placed in this context. We have investigated the processes contributing to the relaxation of a particularly long-lived spin-density wave, which can exist in semiconductor heterostructures with Dresselhaus and Rashba spin-orbit coupling of precisely the same magnitude. We have used a semiclassical spindiffusion equation to study the influence of the Coulomb interaction on the lifetime of this persistent spin helix. We have thus established that, in the presence of perturbations that violate the special symmetry of the problem, electron-electron scattering can have an impact on the relaxation of the spin helix. The resulting temperature-dependent lifetime reproduces the experimentally observed one in a satisfactory manner. It turns out that cubic Dresselhaus spin-orbit coupling is the most important symmetry-breaking element. The Coulomb interaction affects the dynamics of the persistent spin helix also via an Hartree-Fock exchange field. As a consequence, the individual spins precess about the vector of the surrounding local spin density, thus causing a nonlinear dynamics. We have shown that, for an experimentally accessible degree of initial spin polarization, characteristic non-linear effects such as a dramatic increase of lifetime and the appearance of higher harmonics can be expected. Another fascinating solid

Wavefunction and energy of the 1s22sns configuration in a beryllium atom

International Nuclear Information System (INIS)

Huang Shizhong; Ma Kun; Yu Jiaming; Liu Fen

2008-01-01

A new set of trial functions for 1s 2 2sns configurations in a beryllium atom is suggested. A Mathematica program based on the variational method is developed to calculate the wavefunctions and energies of 1s 2 2sns (n = 3–6) configurations in a beryllium atom. Non-relativistic energy, polarization correction and relativistic correction which include mass correction, one-and two-body Darwin corrections, spin-spin contact interaction and orbit-orbit interaction, are calculated respectively. The results are in good agreement with experimental data. (atomic and molecular physics)

Spin-flip transition of L10-type MnPt alloy single crystal studied by neutron scattering

International Nuclear Information System (INIS)

Hama, Hiroaki; Motomura, Ryo; Shinozaki, Tatsuya; Tsunoda, Yorihiko

2007-01-01

Magnetic structure, tetragonality, and the spin-flip transition for an L1 0 -type MnPt ordered alloy were studied by neutron scattering using a single-crystal specimen. Tetragonality of the lattice showed strong correlation with the spin-flip transition. Although the spin-flip transition looks like a gradual change of the easy axis in the temperature range between 580 and 770 K, two modes of magnon-gap peaks with different energies were observed in this transition temperature range. Thus, the crystal consists of two regions with different anisotropy energies and the volume fractions of these regions with different spin directions change gradually with temperature. The tetragonality and spin-flip transition are discussed using the hard-sphere model for atomic radii of Pt and Mn. The Invar effect of Mn atoms is proposed using high- and low-spin transitions of Mn moments in analogy with the two-γ model of Fe moments in FeNi Invar alloy

Optical angular momentum and atoms.

Science.gov (United States)

Franke-Arnold, Sonja

2017-02-28

Any coherent interaction of light and atoms needs to conserve energy, linear momentum and angular momentum. What happens to an atom's angular momentum if it encounters light that carries orbital angular momentum (OAM)? This is a particularly intriguing question as the angular momentum of atoms is quantized, incorporating the intrinsic spin angular momentum of the individual electrons as well as the OAM associated with their spatial distribution. In addition, a mechanical angular momentum can arise from the rotation of the entire atom, which for very cold atoms is also quantized. Atoms therefore allow us to probe and access the quantum properties of light's OAM, aiding our fundamental understanding of light-matter interactions, and moreover, allowing us to construct OAM-based applications, including quantum memories, frequency converters for shaped light and OAM-based sensors.This article is part of the themed issue 'Optical orbital angular momentum'. © 2017 The Author(s).

Single-cell atomic quantum memory for light

International Nuclear Information System (INIS)

Opatrny, Tomas

2006-01-01

Recent experiments demonstrating atomic quantum memory for light [B. Julsgaard et al., Nature 432, 482 (2004)] involve two macroscopic samples of atoms, each with opposite spin polarization. It is shown here that a single atomic cell is enough for the memory function if the atoms are optically pumped with suitable linearly polarized light, and quadratic Zeeman shift and/or ac Stark shift are used to manipulate rotations of the quadratures. This should enhance the performance of our quantum memory devices since less resources are needed and losses of light in crossing different media boundaries are avoided

Quantum incommensurate skyrmion crystals and commensurate to in-commensurate transitions in cold atoms and materials with spin-orbit couplings in a Zeeman field

Science.gov (United States)

Sun, Fadi; Ye, Jinwu; Liu, Wu-Ming

2017-08-01

In this work, we study strongly interacting spinor atoms in a lattice subject to a two dimensional (2d) anisotropic Rashba type of spin orbital coupling (SOC) and an Zeeman field. We find the interplay between the Zeeman field and the SOC provides a new platform to host rich and novel classes of quantum commensurate and in-commensurate phases, excitations and phase transitions. These commensurate phases include two collinear states at low and high Zeeman field, two co-planar canted states at mirror reflected SOC parameters respectively. Most importantly, there are non-coplanar incommensurate Skyrmion (IC-SkX) crystal phases surrounded by the four commensurate phases. New excitation spectra above all the five phases, especially on the IC-SKX phase are computed. Three different classes of quantum commensurate to in-commensurate transitions from the IC-SKX to its four neighboring commensurate phases are identified. Finite temperature behaviors and transitions are discussed. The critical temperatures of all the phases can be raised above that reachable by current cold atom cooling techniques simply by tuning the number of atoms N per site. In view of recent impressive experimental advances in generating 2d SOC for cold atoms in optical lattices, these new many-body phenomena can be explored in the current and near future cold atom experiments. Applications to various materials such as MnSi, {Fe}}0.5 {Co}}0.5Si, especially the complex incommensurate magnetic ordering in Li2IrO3 are given.

Spin effects in strong-field laser-electron interactions

International Nuclear Information System (INIS)

Ahrens, S; Bauke, H; Müller, T-O; Villalba-Chávez, S; Müller, C

2013-01-01

The electron spin degree of freedom can play a significant role in relativistic scattering processes involving intense laser fields. In this contribution we discuss the influence of the electron spin on (i) Kapitza-Dirac scattering in an x-ray laser field of high intensity, (ii) photo-induced electron-positron pair production in a strong laser wave and (iii) multiphoton electron-positron pair production on an atomic nucleus. We show that in all cases under consideration the electron spin can have a characteristic impact on the process properties and their total probabilities. To this end, spin-resolved calculations based on the Dirac equation in the presence of an intense laser field are performed. The predictions from Dirac theory are also compared with the corresponding results from the Klein-Gordon equation.

Electron-spin polarization of photoions produced through photoionization from the laser-excited triplet state of Sr

International Nuclear Information System (INIS)

Yonekura, Nobuaki; Nakajima, Takashi; Matsuo, Yukari; Kobayashi, Tohru; Fukuyama, Yoshimitsu

2004-01-01

We report the detailed experimental study on the production of electron-spin-polarized Sr + ions through one-photon resonant two-photon ionization via laser-excited 5s5p 3 P 1 (M J =+1) of Sr atoms produced by laser-ablation. We have experimentally confirmed that the use of laser-ablation for the production of Sr atoms prior to photoionization does not affect the electron-spin polarization. We have found that the degree of electron-spin polarization is 64±9%, which is in good agreement with our recent theoretical prediction. As we discuss in detail, we infer, from a simple analysis, that photoelectrons, being the counterpart of electron-spin-polarized Sr + ions, have approximately the same degree of electron-spin polarization. Our experimental results demonstrate that the combined use of laser-ablation technique and pulsed lasers for photoionization would be a compact and effective way to realize a pulsed source for spin-polarized ions and electrons for the studies of various spin-dependent dynamics in chemical physics

Spatial Multiplexing of Atom-Photon Entanglement Sources using Feedforward Control and Switching Networks.

Science.gov (United States)

Tian, Long; Xu, Zhongxiao; Chen, Lirong; Ge, Wei; Yuan, Haoxiang; Wen, Yafei; Wang, Shengzhi; Li, Shujing; Wang, Hai

2017-09-29

The light-matter quantum interface that can create quantum correlations or entanglement between a photon and one atomic collective excitation is a fundamental building block for a quantum repeater. The intrinsic limit is that the probability of preparing such nonclassical atom-photon correlations has to be kept low in order to suppress multiexcitation. To enhance this probability without introducing multiexcitation errors, a promising scheme is to apply multimode memories to the interface. Significant progress has been made in temporal, spectral, and spatial multiplexing memories, but the enhanced probability for generating the entangled atom-photon pair has not been experimentally realized. Here, by using six spin-wave-photon entanglement sources, a switching network, and feedforward control, we build a multiplexed light-matter interface and then demonstrate a ∼sixfold (∼fourfold) probability increase in generating entangled atom-photon (photon-photon) pairs. The measured compositive Bell parameter for the multiplexed interface is 2.49±0.03 combined with a memory lifetime of up to ∼51  μs.

Spin tunnelling dynamics for spin-1 Bose-Einstein condensates in a swept magnetic field

International Nuclear Information System (INIS)

Wang Guanfang; Fu Libin; Liu Jie

2008-01-01

We investigate the spin tunnelling of spin-1 Bose-Einstein condensates in a linearly swept magnetic field with a mean-field treatment. We focus on the two typical alkali Bose atoms 87 Rb and 23 Na condensates and study their tunnelling dynamics according to the sweep rates of the external magnetic fields. In the adiabatic (i.e. slowly sweeping) and sudden (i.e. fast sweeping) limits, no tunnelling is observed. For the case of moderate sweep rates, the tunnelling dynamics is found to be very sensitive to the sweep rates, so the plots of tunnelling probability versus sweep rate only become resolvable at a resolution of 10 -4 G s -1 . Moreover, a conserved quantity standing for the magnetization in experiments is found to affect dramatically the dynamics of the spin tunnelling. Theoretically we have given a complete interpretation of the above findings, and our studies could stimulate the experimental study of spinor Bose-Einstein condensates

STM studies of an atomic-scale gate electrode formed by a single charged vacancy in GaAs

Science.gov (United States)

Lee, Donghun; Daughton, David; Gupta, Jay

2009-03-01

Electric-field control of spin-spin interactions at the atomic level is desirable for the realization of spintronics and spin-based quantum computation. Here we demonstrate the realization of an atomic-scale gate electrode formed by a single charged vacancy on the GaAs(110) surface[1]. We can position these vacancies with atomic precision using the tip of a home-built, low temperature STM. Tunneling spectroscopy of single Mn acceptors is used to quantify the electrostatic field as a function of distance from the vacancy. Single Mn acceptors are formed by substituting Mn adatoms for Ga atoms in the first layer of the p-GaAs(110) surface[2]. Depending on the distance, the in-gap resonance of single Mn acceptors can shift as much as 200meV. Our data indicate that the electrostatic field decays according to a screened Coulomb potential. The charge state of the vacancy can be switched to neutral, as evidenced by the Mn resonance returning to its unperturbed position. Reversible control of the local electric field as well as charged states of defects in semiconductors can open new insights such as realizing an atomic-scale gate control and studying spin-spin interactions in semiconductors. http://www.physics.ohio-state.edu/sim jgupta [1] D. Lee and J.A. Gupta (in preparation) [2] D. Kitchen et al., Nature 442, 436-439 (2006)

Precision polarization measurements of atoms in a far-off-resonance optical dipole trap

International Nuclear Information System (INIS)

Fang, F.; Vieira, D. J.; Zhao, X.

2011-01-01

Precision measurement of atomic and nuclear polarization is an essential step for beta-asymmetry measurement of radioactive atoms. In this paper, we report the polarization measurement of Rb atoms in an yttrium-aluminum-garnet (YAG) far-off-resonance optical dipole trap. We have prepared a cold cloud of polarized Rb atoms in the YAG dipole trap by optical pumping and achieved an initial nuclear polarization of up to 97.2(5)%. The initial atom distribution in different Zeeman levels is measured by using a combination of microwave excitation, laser pushing, and atomic retrap techniques. The nuclear-spin polarization is further purified to 99.2(2)% in 10 s and maintained above 99% because the two-body collision loss rate between atoms in mixed spin states is greater than the one-body trap loss rate. Systematic effects on the nuclear polarization, including the off-resonance Raman scattering, magnetic field gradient, and background gas collisions, are discussed.

Spin Polarization Inversion at Benzene-Absorbed Fe4N Surface

KAUST Repository

Zhang, Qian; Mi, Wenbo; Wang, Xiaocha; Wang, Xuhui

2015-01-01

We report a first-principle study on electronic structure and simulation of the spin-polarized scanning tunneling microscopy graphic of a benzene/Fe4N interface. Fe4N is a compound ferromagnet suitable for many spintronic applications. We found that, depending on the particular termination schemes and interface configurations, the spin polarization on the benzene surface shows a rich variety of properties ranging from cosine-type oscillation to polarization inversion. Spin-polarization inversion above benzene is resulting from the hybridizations between C pz and the out-of-plane d orbitals of Fe atom.

Spin Polarization Inversion at Benzene-Absorbed Fe4N Surface

KAUST Repository

Zhang, Qian

2015-05-27

We report a first-principle study on electronic structure and simulation of the spin-polarized scanning tunneling microscopy graphic of a benzene/Fe4N interface. Fe4N is a compound ferromagnet suitable for many spintronic applications. We found that, depending on the particular termination schemes and interface configurations, the spin polarization on the benzene surface shows a rich variety of properties ranging from cosine-type oscillation to polarization inversion. Spin-polarization inversion above benzene is resulting from the hybridizations between C pz and the out-of-plane d orbitals of Fe atom.

Degenerate quantum gases with spin-orbit coupling: a review.

Science.gov (United States)

Zhai, Hui

2015-02-01

This review focuses on recent developments in synthetic spin-orbit (SO) coupling in ultracold atomic gases. Two types of SO coupling are discussed. One is Raman process induced coupling between spin and motion along one of the spatial directions and the other is Rashba SO coupling. We emphasize their common features in both single-particle and two-body physics and the consequences of both in many-body physics. For instance, single particle ground state degeneracy leads to novel features of superfluidity and a richer phase diagram; increased low-energy density-of-state enhances interaction effects; the absence of Galilean invariance and spin-momentum locking gives rise to intriguing behaviours of superfluid critical velocity and novel quantum dynamics; and the mixing of two-body singlet and triplet states yields a novel fermion pairing structure and topological superfluids. With these examples, we show that investigating SO coupling in cold atom systems can, enrich our understanding of basic phenomena such as superfluidity, provide a good platform for simulating condensed matter states such as topological superfluids and more importantly, result in novel quantum systems such as SO coupled unitary Fermi gas and high spin quantum gases. Finally we also point out major challenges and some possible future directions.

EPR spin probe and spin label studies of some low molecular and polymer micelles

Science.gov (United States)

Wasserman, A. M.; Kasaikin, V. A.; Timofeev, V. P.

1998-12-01

The rotational mobility of spin probes of different shape and size in low molecular and polymer micelles has been studied. Several probes having nitroxide fragment localized either in the vicinity of micelle interface or in the hydrocarbon core have been used. Upon increasing the number of carbon atoms in hydrocarbon chain of detergent from 7 to 13 (sodium alkyl sulfate micelles) or from 12 to 16 (alkyltrimethylammonium bromide micelles) the rotational mobility of spin probes is decreased by the factor 1.5-2.0. The spin probe rotational mobility in polymer micelles (the complexes of alkyltrimethylammonium bromides and polymethacrylic or polyacrylic acids) is less than mobility in free micelles of the same surfactants. The study of EPR-spectra of spin labeled polymethacrylic acid (PMA) indicated that formation of water soluble complexes of polymer and alkyltrimethylammonium bromides in alkaline solutions (pH 9) does not affect the polymer segmental mobility. On the other hand, the polymer complexes formation in slightly acidic water solution (pH 6) breaks down the compact PMA conformation, thus increasing the polymer segmental mobility. Possible structures of polymer micelles are discussed.

Quantum phases of electric dipole ensembles in atom chips

International Nuclear Information System (INIS)

Pachos, Jiannis K.

2005-01-01

We present how a phase factor is generated when an electric dipole moves along a closed trajectory inside a magnetic field gradient. The similarity of this situation with charged particles in a magnetic field can be employed to simulate condensed matter models, such as the quantum Hall effect and chiral spin Hamiltonians, with ultra cold atoms integrated on atom chips. To illustrate this we consider a triangular configuration of a two-dimensional optical lattice, where the chiral spin Hamiltonian σ-> i -bar σ-> j xσ-> k can be generated between any three neighbours on a lattice yielding an experimentally implementable chiral ground state

Determination of nuclear spins of short-lived isotopes by laser induced fluorescence

International Nuclear Information System (INIS)

Buchinger, F.; Dabkiewicz, P.; Kremmling, H.; Kuehl, T.; Mueller, A.C.; Schuessler, H.A.

1980-01-01

The spins of several nuclear ground and isomeric states have been measured for a number of mercury isotopes. The fluorescent light from the 6s6p 3 P 1 state is observed at 2537 Angstroem after excitation with the frequency doubled output of a pulsed dye laser. Four different laser induced fluorescence techniques were tested for their applicability: double resonance, Hanle effect, time delayed integral Hanle beats, and time resolved quantum beats. The sensitivity and selectivity of these models are compared with emphasis on the determination of spins of nuclei far from beta-stability, where short half lives and low production yields restrict the number of available atoms. The experiments were carried out on-line with the ISOLDE isotope separator at CERN at densities as low as 10 6 atoms/cm 3 . Results for the very neutron deficient high spin mercury isomers with half lives of several seconds, but also for the ground states of the abundant low spin stable mercury isotopes, are given as examples. The test measurements determined the nuclear spins of the odd sup(185m-191m)Hg isomers to be I = 13/2. (orig.)

Episodic Spin-up and Spin-down Torque on Earth

Science.gov (United States)

Slabinski, Victor J.; Mendonca, Antonio A.

2018-04-01

Variations in Earth rotation angle are traditionally expressed by the time difference (ΔT=TT-UT1) between Terrestrial Time (TT) as told by atomic clocks and Universal Time UT1, the time variable used by the Earth-rotation formula. A plot of ΔT versus TT over the past 160 years shows a continuous curve with approximate straight-line segments with different spans of order ~20 years. Removing the tidal and seasonal variations from the data gives these line segments which represent the “decadal variations” in Earth rotation.The slope of a straight-line segment is proportional to the departure of Earth rotation rate from a reference value at the time. The change in slope over the relatively short time between segments indicates an episodic spin-up or spin-down in Earth rotation. The daily combination of VLBI, SLR, and other modern data available since 1973 gives us accurate, daily values of ΔT and the corresponding LOD (Length Of Day) values during these episodes. These allow us to determine the rotational acceleration occurring then.The three largest spin-speed changes found during the VLBI era have the following characteristics:Episode _____________ Duration__ ΔLOD__LOD Rate1983 Dec 30-1984 Jan 28 ... 29 d ...-0.65 ms ..-8.3 ms/y ..........spin-up1989 Mar 15-1989 May 23 ...69 d ....0.68 .......+3.6 ..............spin-down1994 Jan 21-2001 Apr 01 ... 6.5 y ...-2.2 .........-0.36 ..extended spin-upFor the first two episodes listed, we find the acceleration grows from zero (or at least a relatively small value) to its extreme value in ~1 day, stays approximately constant at this value for 29 or 69 days, and then decays back to zero over ~1 day. The acceleration, while it occurs, gives an LOD rate much greater than the 0.02 ms/y rate from tidal friction.The third episode shows that occasionally a several-year-long episode occurs. The acceleration magnitude is smaller but can make a larger total change in LOD (and spin rate). Tidal friction requires >100 y to equal

From few to many. Ultracold atoms in reduced dimensions

International Nuclear Information System (INIS)

Wenz, Andre Niklas

2013-01-01

This thesis reports on experimental studies exploring few and many-body physics of ultracold Bose and Fermi gases with reduced dimensionality. These experiments illustrate the versatility and great amount of control over the particle number, the interaction and other degrees of freedom, like the spin, that these generic quantum systems offer. In the first part of this thesis, we use quasi one-dimensional few-particle systems of one to ten fermionic atoms to investigate the crossover from few to many-body physics. This is achieved by measuring the interaction energy between a single impurity atom in a state vertical stroke ↓ right angle which repulsively interacts with an increasing number of majority atoms in a state vertical stroke ↑ right angle. We find that the system quickly approaches the results from the many-body theory, which describes the behavior of a single impurity immersed in a Fermi sea of an infinite number of majority particles. The second part of this thesis presents studies of the time evolution of a bosonic F=1 spinor BEC of 87 Rb atoms. In this system, we investigate the emergence and coarsening of ferromagnetic spin textures from initially unmagnetized samples. While the ferromagnetic domains grow, we observe the development of a spin space anisotropy which is in agreement with the predicted phase-diagram. The last part of this thesis presents our first steps towards the investigation of phase coherence of quasi two-dimensional quantum gases in the crossover from bosonic molecules to fermionic atoms.

From few to many. Ultracold atoms in reduced dimensions

Energy Technology Data Exchange (ETDEWEB)

Wenz, Andre Niklas

2013-12-19

This thesis reports on experimental studies exploring few and many-body physics of ultracold Bose and Fermi gases with reduced dimensionality. These experiments illustrate the versatility and great amount of control over the particle number, the interaction and other degrees of freedom, like the spin, that these generic quantum systems offer. In the first part of this thesis, we use quasi one-dimensional few-particle systems of one to ten fermionic atoms to investigate the crossover from few to many-body physics. This is achieved by measuring the interaction energy between a single impurity atom in a state vertical stroke ↓ right angle which repulsively interacts with an increasing number of majority atoms in a state vertical stroke ↑ right angle. We find that the system quickly approaches the results from the many-body theory, which describes the behavior of a single impurity immersed in a Fermi sea of an infinite number of majority particles. The second part of this thesis presents studies of the time evolution of a bosonic F=1 spinor BEC of {sup 87}Rb atoms. In this system, we investigate the emergence and coarsening of ferromagnetic spin textures from initially unmagnetized samples. While the ferromagnetic domains grow, we observe the development of a spin space anisotropy which is in agreement with the predicted phase-diagram. The last part of this thesis presents our first steps towards the investigation of phase coherence of quasi two-dimensional quantum gases in the crossover from bosonic molecules to fermionic atoms.

Protecting nickel with graphene spin-filtering membranes: A single layer is enough

Energy Technology Data Exchange (ETDEWEB)

Martin, M.-B.; Dlubak, B.; Piquemal-Banci, M.; Collin, S.; Petroff, F.; Anane, A.; Fert, A.; Seneor, P. [Unité Mixte de Physique CNRS/Thales, 1 Avenue Augustin Fresnel, 91767 Palaiseau, France and Université Paris Sud, 91405 Orsay (France); Weatherup, R. S.; Hofmann, S.; Robertson, J. [Department of Engineering, University of Cambridge, Cambridge CB21PZ (United Kingdom); Yang, H. [IBS Center for Integrated Nanostructure Physics (CINAP), Institute for Basic Science, Sungkyunkwan University, Suwon 440-746 (Korea, Republic of); Department of Energy Science, Sungkyunkwan University, Suwon 440-746 (Korea, Republic of); Blume, R. [Helmholtz-Zentrum Berlin fur Materialien und Energie, 12489 Berlin (Germany); Schloegl, R. [Department of Inorganic Chemistry, Fritz Haber Institute of the Max Planck Society, Faradayweg 4-6, 14195 Berlin (Germany)

2015-07-06

We report on the demonstration of ferromagnetic spin injectors for spintronics which are protected against oxidation through passivation by a single layer of graphene. The graphene monolayer is directly grown by catalytic chemical vapor deposition on pre-patterned nickel electrodes. X-ray photoelectron spectroscopy reveals that even with its monoatomic thickness, monolayer graphene still efficiently protects spin sources against oxidation in ambient air. The resulting single layer passivated electrodes are integrated into spin valves and demonstrated to act as spin polarizers. Strikingly, the atom-thick graphene layer is shown to be sufficient to induce a characteristic spin filtering effect evidenced through the sign reversal of the measured magnetoresistance.

Coherent manipulation of spin correlations in the Hubbard model

Science.gov (United States)

Wurz, N.; Chan, C. F.; Gall, M.; Drewes, J. H.; Cocchi, E.; Miller, L. A.; Pertot, D.; Brennecke, F.; Köhl, M.

2018-05-01

We coherently manipulate spin correlations in a two-component atomic Fermi gas loaded into an optical lattice using spatially and time-resolved Ramsey spectroscopy combined with high-resolution in situ imaging. This technique allows us not only to imprint spin patterns but also to probe the static magnetic structure factor at an arbitrary wave vector, in particular, the staggered structure factor. From a measurement along the diagonal of the first Brillouin zone of the optical lattice, we determine the magnetic correlation length and the individual spatial spin correlators. At half filling, the staggered magnetic structure factor serves as a sensitive thermometer, which we employ to study the equilibration in the spin and density sector during a slow quench of the lattice depth.

Observation of Spin Superfluidity in a Bose Gas Mixture

Science.gov (United States)

Fava, Eleonora; Bienaimé, Tom; Mordini, Carmelo; Colzi, Giacomo; Qu, Chunlei; Stringari, Sandro; Lamporesi, Giacomo; Ferrari, Gabriele

2018-04-01

The spin dynamics of a harmonically trapped Bose-Einstein condensed binary mixture of sodium atoms is experimentally investigated at finite temperature. In the collisional regime the motion of the thermal component is shown to be damped because of spin drag, while the two condensates exhibit a counterflow oscillation without friction, thereby providing direct evidence for spin superfluidity. Results are also reported in the collisionless regime where the spin components of both the condensate and thermal part oscillate without damping, their relative motion being driven by a mean-field effect. We also measure the static polarizability of the condensed and thermal parts and we find a large increase of the condensate polarizability with respect to the T =0 value, in agreement with the predictions of theory.

Orientation of Ar(3P2) atoms by laser optical pumping

International Nuclear Information System (INIS)

Giberson, K.W.; Hart, M.W.; Hammond, M.S.; Dunning, F.B.; Walters, G.K.

1984-01-01

A beam of argon metastable atoms with a high degree of electron-spin polarization has been produced by optical pumping using an Oxazine 750 dye laser. The beam is suitable for the study of electron spin and orbital orientation dependences in a variety of collision processes

Generating spin squeezing states and Greenberger-Horne-Zeilinger entanglement using a hybrid phonon-spin ensemble in diamond

Science.gov (United States)

Xia, Keyu; Twamley, Jason

2016-11-01

Quantum squeezing and entanglement of spins can be used to improve the sensitivity in quantum metrology. Here we propose a scheme to create collective coupling of an ensemble of spins to a mechanical vibrational mode actuated by an external magnetic field. We find an evolution time where the mechanical motion decouples from the spins, and the accumulated geometric phase yields a squeezing of 5.9 dB for 20 spins. We also show the creation of a Greenberger-Horne-Zeilinger spin state for 20 spins with a fidelity of ˜0.62 at cryogenic temperature. The numerical simulations show that the geometric-phase-based scheme is mostly immune to thermal mechanical noise.

Continuous Faraday measurement of spin precession without light shifts

Science.gov (United States)

Jasperse, M.; Kewming, M. Â. J.; Fischer, S. Â. N.; Pakkiam, P.; Anderson, R. Â. P.; Turner, L. Â. D.

2017-12-01

We describe a dispersive Faraday optical probe of atomic spin which performs a weak measurement of spin projection of a quantum gas continuously for more than one second. To date, focusing bright far-off-resonance probes onto quantum gases has proved invasive due to strong scalar and vector light shifts exerting dipole and Stern-Gerlach forces. We show that tuning the probe near the magic-zero wavelength at 790 nm between the fine-structure doublet of 87Rb cancels the scalar light shift, and careful control of polarization eliminates the vector light shift. Faraday rotations due to each fine-structure line reinforce at this wavelength, enhancing the signal-to-noise ratio for a fixed rate of probe-induced decoherence. Using this minimally invasive spin probe, we perform microscale atomic magnetometry at high temporal resolution. Spectrogram analysis of the Larmor precession signal of a single spinor Bose-Einstein condensate measures a time-varying magnetic field strength with 1 μ G accuracy every 5 ms; or, equivalently, makes more than 200 successive measurements each at 10 pT /√{Hz } sensitivity.

Spin squeezing and light entanglement in Coherent Population Trapping

DEFF Research Database (Denmark)

Dantan, Aurelien Romain; Cviklinski, Jean; Giacobino, Elisabeth

2006-01-01

We show that strong squeezing and entanglement can be generated at the output of a cavity containing atoms interacting with two fields in a coherent population trapping situation, on account of a nonlinear Faraday effect experienced by the fields close to a dark-state resonance in a cavity....... Moreover, the cavity provides a feedback mechanism allowing to reduce the quantum fluctuations of the ground state spin, resulting in strong steady state spin squeezing....

Electron spin resonance in YbRh2Si2: local-moment, unlike-spin and quasiparticle descriptions.

Science.gov (United States)

Huber, D L

2012-06-06

Electron spin resonance (ESR) in the Kondo lattice compound YbRh(2)Si(2) has stimulated discussion as to whether the low-field resonance outside the Fermi liquid regime in this material is more appropriately characterized as a local-moment phenomenon or one that requires a Landau quasiparticle interpretation. In earlier work, we outlined a collective mode approach to the ESR that involves only the local 4f moments. In this paper, we extend the collective mode approach to a situation where there are two subsystems of unlike spins: the pseudospins of the ground multiplet of the Yb ions and the spins of the itinerant conduction electrons. We assume a weakly anisotropic exchange interaction between the two subsystems. With suitable approximations our expression for the g-factor also reproduces that found in recent unlike-spin quasiparticle calculations. It is pointed out that the success of the local-moment approach in describing the resonance is due to the fact that the susceptibility of the Yb subsystem dominates that of the conduction electrons with the consequence that the relative shift in the resonance frequency predicted by the unlike-spin models (and absent in the local-moment models) is ≪ 1. The connection with theoretical studies of a two-component model with like spins is also discussed.

SPINning parallel systems software

International Nuclear Information System (INIS)

Matlin, O.S.; Lusk, E.; McCune, W.

2002-01-01

We describe our experiences in using Spin to verify parts of the Multi Purpose Daemon (MPD) parallel process management system. MPD is a distributed collection of processes connected by Unix network sockets. MPD is dynamic processes and connections among them are created and destroyed as MPD is initialized, runs user processes, recovers from faults, and terminates. This dynamic nature is easily expressible in the Spin/Promela framework but poses performance and scalability challenges. We present here the results of expressing some of the parallel algorithms of MPD and executing both simulation and verification runs with Spin

ESR study on hydrogen-atom abstraction in cryogenic organic solids

International Nuclear Information System (INIS)

Ichikawa, Tsuneki

1995-01-01

The present paper summarizes our recent results on the hydrogen-atom abstraction from protiated alkane molecule by deuterium atoms in cryogenic deuterated organic solids, obtained by the X-band ESR and electron spin-echo measurements of the product alkyl radicals at cryogenic temperatures. (J.P.N.)

Double-decker phthalocyanine complex: Scanning tunneling microscopy study of film formation and spin properties

Science.gov (United States)

Komeda, Tadahiro; Katoh, Keiichi; Yamashita, Masahiro

2014-05-01

We review recent studies of double-decker and triple-decker phthalocyanine (Pc) molecules adsorbed on surfaces in terms of the bonding configuration, electronic structure and spin state. The Pc molecule has been studied extensively in surface science. A Pc molecule can contain various metal atoms at the center, and the class of the molecule is called as metal phthalocyanine (MPc). If the center metal has a large radius, like as lanthanoid metals, it becomes difficult to incorporate the metal atom inside of the Pc ring. Pc ligands are placed so as to sandwich the metal atom, where the metal atom is placed out of the Pc plane. The molecule in this configuration is called as a multilayer-decker Pc molecule. After the finding that the double-decker Pc lanthanoid complex shows single-molecule magnet (SMM) behavior, it has attracted a large attention. This is partly due to a rising interest for the ‘molecular spintronics’, in which the freedoms of spin and charge of an electron are applied to the quantum process of information. SMMs represent a class of compounds in which a single molecule behaves as a magnet. The reported blocking temperature, below which a single SMM molecule works as an quantum magnet, has been increasing with the development in the molecular design and synthesis techniques of multiple-decker Pc complex. However, even the bulk properties of these molecules are promising for the use of electronic materials, the films of multi-decker Pc molecules is less studied than those for the MPc molecules. An intriguing structural property is expected for the multi-decker Pc molecules since the Pc planes are linked by metal atoms. This gives an additional degree of freedom to the rotational angle between the two Pc ligands, and they can make a wheel-like symmetric rotation. Due to a simple and well-defined structure of a multi-decker Pc complex, the molecule can be a model molecule for molecular machine studies. The multi-decker Pc molecules can provide

Spin resolved electronic transport through N@C20 fullerene molecule between Au electrodes: A first principles study

Science.gov (United States)

Caliskan, Serkan

2018-05-01

Using first principles study, through Density Functional Theory combined with Non Equilibrium Green's Function Formalism, electronic properties of endohedral N@C20 fullerene molecule joining Au electrodes (Au-N@C20) was addressed in the presence of spin property. The electronic transport behavior across the Au-N@C20 molecular junction was investigated by spin resolved transmission, density of states, molecular orbitals, differential conductance and current-voltage (I-V) characteristics. Spin asymmetric variation was clearly observed in the results due to single N atom encapsulated in the C20 fullerene cage, where the N atom played an essential role in the electronic behavior of Au-N@C20. This N@C20 based molecular bridge, exhibiting a spin dependent I-V variation, revealed a metallic behavior within the bias range from -1 V to 1 V. The induced magnetic moment, spin polarization and other relevant quantities associated with the spin resolved transport were elucidated.

Atomic spin-chain realization of a model for quantum criticality

NARCIS (Netherlands)

Toskovic, R.; van den Berg, R.; Spinelli, A.; Eliens, I.S.; van den Toorn, B.; Bryant, B.; Caux, J.-S.; Otte, A.F.

The ability to manipulate single atoms has opened up the door to constructing interesting and useful quantum structures from the ground up. On the one hand, nanoscale arrangements of magnetic atoms are at the heart of future quantum computing and spintronic devices; on the other hand, they can be

Quantum model of a solid-state spin qubit: Ni cluster on a silicon surface by the generalized spin Hamiltonian and X-ray absorption spectroscopy investigations

Science.gov (United States)

Farberovich, Oleg V.; Mazalova, Victoria L.; Soldatov, Alexander V.

2015-11-01

We present here the quantum model of a Ni solid-state electron spin qubit on a silicon surface with the use of a density-functional scheme for the calculation of the exchange integrals in the non-collinear spin configurations in the generalized spin Hamiltonian (GSH) with the anisotropic exchange coupling parameters linking the nickel ions with a silicon substrate. In this model the interaction of a spin qubit with substrate is considered in GSH at the calculation of exchange integrals Jij of the nanosystem Ni7-Si in the one-electron approach taking into account chemical bonds of all Si-atoms of a substrate (environment) with atoms of the Ni7-cluster. The energy pattern was found from the effective GSH Hamiltonian acting in the restricted spin space of the Ni ions by the application of the irreducible tensor operators (ITO) technique. In this paper we offer the model of the quantum solid-state N-spin qubit based on the studying of the spin structure and the spin-dynamics simulations of the 3d-metal Ni clusters on the silicon surface. The solution of the problem of the entanglement between spin states in the N-spin systems is becoming more interesting when considering clusters or molecules with a spectral gap in their density of states. For quantifying the distribution of the entanglement between the individual spin eigenvalues (modes) in the spin structure of the N-spin system we use the density of entanglement (DOE). In this study we have developed and used the advanced high-precision numerical techniques to accurately assess the details of the decoherence process governing the dynamics of the N-spin qubits interacting with a silicon surface. We have studied the Rabi oscillations to evaluate the N-spin qubits system as a function of the time and the magnetic field. We have observed the stabilized Rabi oscillations and have stabilized the quantum dynamical qubit state and Rabi driving after a fixed time (0.327 μs). The comparison of the energy pattern with the

Anomalous conductance oscillations and half-metallicity in atomic Ag-O chains

DEFF Research Database (Denmark)

Strange, Mikkel; Thygesen, Kristian Sommer; Sethna, James P

2008-01-01

. The conductances of the chains exhibit weak even-odd oscillations around an anomalously low value of 0.1G(0) (G(0) = 2e(2)/h) which coincide with the averaged experimental conductance in the long chain limit. The unusual conductance properties are explained in terms of a resonating-chain model, which takes...... the reflection probability and phase shift of a single bulk-chain interface as the only input. The model also explains the conductance oscillations for other metallic chains.......Using spin density functional theory, we study the electronic and magnetic properties of atomically thin, suspended chains containing silver and oxygen atoms in an alternating sequence. Chains longer than 4 atoms develop a half-metallic ground state implying fully spin-polarized charge carriers...