Efficient Multiparticle Entanglement via Asymmetric Rydberg Blockade

DEFF Research Database (Denmark)

Saffman, Mark; Mølmer, Klaus

2009-01-01

We present an efficient method for producing N particle entangled states using Rydberg blockade interactions. Optical excitation of Rydberg states that interact weakly, yet have a strong coupling to a second control state is used to achieve state dependent qubit rotations in small ensembles. On t....... On the basis of quantitative calculations, we predict that an entangled quantum superposition state of eight atoms can be produced with a fidelity of 84% in cold Rb atoms.......We present an efficient method for producing N particle entangled states using Rydberg blockade interactions. Optical excitation of Rydberg states that interact weakly, yet have a strong coupling to a second control state is used to achieve state dependent qubit rotations in small ensembles...

Implementation of quantum logic gates via Stark-tuned Förster resonance in Rydberg atoms

Science.gov (United States)

Huang, Xi-Rong; Hu, Chang-Sheng; Shen, Li-Tuo; Yang, Zhen-Biao; Wu, Huai-Zhi

2018-02-01

We present a scheme for implementation of controlled-Z and controlled-NOT gates via rapid adiabatic passage and Stark-tuned Förster resonance. By sweeping the Förster resonance once without passing through it and adiabatically tuning the angle-dependent Rydberg-Rydberg interaction of the dipolar nature, the system can be effectively described by a two-level system with the adiabatic theorem. The single adiabatic passage leads to a gate fidelity as high as 0.999 and a greatly reduced gate operation time. We investigate the scheme by considering an actual atomic level configuration with rubidium atoms, where the fidelity of the controlled-Z gate is still higher than 0.99 under the influence of the Zeeman effect.

Spectroscopy of strontium Rydberg states using electromagnetically induced transparency

International Nuclear Information System (INIS)

Mauger, S; Millen, J; Jones, M P A

2007-01-01

We report on the all-optical detection of Rydberg states in an effusive atomic beam of strontium atoms using electromagnetically induced transparency (EIT). Using narrow-linewidth CW lasers we obtain an EIT linewidth of 5 MHz. To illustrate the high spectroscopic resolution offered by this method, we have measured isotope shifts of the 5s18d 1 D 2 and 5s19s 1 S 0 Rydberg states. This technique could be applied to high-resolution, non-destructive measurements of ultra-cold Rydberg gases and plasmas. (fast track communication)

Autoionizing Rydberg series in alkali atoms

International Nuclear Information System (INIS)

Kulov, M.A.; Ivanov, V.K.; Cherepkov, N.A.

2004-01-01

Full text: The results of many-body calculations of autoionizing resonance structure in neutral potassium, rubidium and cesium associated with the ns 2 np 6 (n+1)s → nsnp 6 (n+1)smp Rydberg excitations are presented. The numerical method based on the Many-Body Perturbation Theory takes into account the dynamic polarization and screening of electron-electron interaction by collective motion of the whole electronic system. The many-electron effects are shown to determine the resonance shapes. The numerically obtained cross section for photoionization of 3p electrons in neutral K in the vicinity of the 3s threshold is presented. The structure has the complex shape of 3s → mp resonances due to different behavior of electrons with the opposite spin projections

Observation of electric quadrupole transitions to Rydberg nd states of ultracold rubidium atoms

NARCIS (Netherlands)

Tong, D.; Farooqi, S.M.; Kempen, van E.G.M.; Pavlovic, Z.; Stanojevic, J.; Coté, R.; Eyler, E.E.; Gould, P.L.

2009-01-01

We report the observation of dipole-forbidden, but quadrupole-allowed, one-photon transitions to high-Rydberg states in Rb. Using pulsed uv excitation of ultracold atoms in a magneto-optical trap, we excite 5s¿nd transitions over a range of principal quantum numbers n=27–59. Compared to

CrossRef Large numbers of cold positronium atoms created in laser-selected Rydberg states using resonant charge exchange

CERN Document Server

McConnell, R; Kolthammer, WS; Richerme, P; Müllers, A; Walz, J; Grzonka, D; Zielinski, M; Fitzakerley, D; George, MC; Hessels, EA; Storry, CH; Weel, M

2016-01-01

Lasers are used to control the production of highly excited positronium atoms (Ps*). The laser light excites Cs atoms to Rydberg states that have a large cross section for resonant charge-exchange collisions with cold trapped positrons. For each trial with 30 million trapped positrons, more than 700 000 of the created Ps* have trajectories near the axis of the apparatus, and are detected using Stark ionization. This number of Ps* is 500 times higher than realized in an earlier proof-of-principle demonstration (2004 Phys. Lett. B 597 257). A second charge exchange of these near-axis Ps* with trapped antiprotons could be used to produce cold antihydrogen, and this antihydrogen production is expected to be increased by a similar factor.

The search For Closed Orbits Of General Rydberg Atoms in External Fields And Their Classification

International Nuclear Information System (INIS)

Carboni, R.

1997-01-01

A program of high precision that find closed orbits for the classical motion of the electron of general Rydberg atoms in crossed magnetic and electric fields is explained. Investigations of the influence of the ionic core on the electronic trajectories using a phenomenological model potential were done. Additional closed orbits that are not present in hydrogen atoms and that seem to be composed of hydrogenic orbits were found. The stability and formation of orbits are explained. Using the generalized closed-orbit theory, the scaled recurrence spectra for rubidium Rydberg atoms were calculated. The results are in good agreement with reported experiments. Two important features of the expectra can be explained by classical core scattering: The additional non-hydrogenic resonances associated to composite orbits and the vanishing of hydrogenic resonances related to closed or whose trajectories approach the core. (Author) [es

Radio-over-fiber using an optical antenna based on Rydberg states of atoms

Science.gov (United States)

Deb, A. B.; Kjærgaard, N.

2018-05-01

We provide an experimental demonstration of a direct fiber-optic link for RF transmission ("radio-over-fiber") using a sensitive optical antenna based on a rubidium vapor cell. The scheme relies on measuring the transmission of laser light at an electromagnetically induced transparency resonance that involves highly excited Rydberg states. By dressing pairs of Rydberg states using microwave fields that act as local oscillators, we encoded RF signals in the optical frequency domain. The light carrying the information is linked via a virtually lossless optical fiber to a photodetector where the signal is retrieved. We demonstrate a signal bandwidth in excess of 1 MHz limited by the available coupling laser power and atomic optical density. Our sensitive, non-metallic and readily scalable optical antenna for microwaves allows extremely low-levels of optical power (˜1 μW) throughput in the fiber-optic link. It offers a promising future platform for emerging wireless network infrastructures.

Rydberg states

International Nuclear Information System (INIS)

Brouillard, F.

1983-01-01

This chapter considers the formation of Rydberg atoms; their radiative decay; their behavior in electric and electromagnetic fields; and their collisions with atoms and ions. Discusses electron capture into high excited states; laser excitation of Rydberg states; Stark shift and Stark mixing; field ionization; ionization in oscillating fields; thermal collisions of Rydberg atoms; fast collisions of Rydberg atoms; n-changing collisions; and charge exchange. Points out that a large amount of experimental work has been done on collisions of Rydberg atoms with neutral perturbers at thermal energies, and most of it concerns the destruction of Rydberg alkali atoms in collisions with rare gases

Electromagnetically induced grating with Rydberg atoms

Science.gov (United States)

Asghar, Sobia; Ziauddin, Qamar, Shahid; Qamar, Sajid

2016-09-01

We present a scheme to realize electromagnetically induced grating in an ensemble of strongly interacting Rydberg atoms, which act as superatoms due to the dipole blockade mechanism. The ensemble of three-level cold Rydberg-dressed (87Rb) atoms follows a cascade configuration where a strong standing-wave control field and a weak probe pulse are employed. The diffraction intensity is influenced by the strength of the probe intensity, the control field strength, and the van der Waals (vdW) interaction. It is noticed that relatively large first-order diffraction can be obtained for low-input intensity with a small vdW shift and a strong control field. The scheme can be considered as an amicable solution to realize the atomic grating at the microscopic level, which can provide background- and dark-current-free diffraction.

Provisional Peer-Reviewed Toxicity Values for Rubidium Compounds (Rubidium Chloride)

Science.gov (United States)

This is a PPRTV for Rubidium Compounds submitted to the Superfund Program.This assessment supports multiple isomers (see related links) and this page is about the chemical rubidium chloride, CASRN 7791-11-9.

Non-adiabatic quantum state preparation and quantum state transport in chains of Rydberg atoms

Science.gov (United States)

Ostmann, Maike; Minář, Jiří; Marcuzzi, Matteo; Levi, Emanuele; Lesanovsky, Igor

2017-12-01

Motivated by recent progress in the experimental manipulation of cold atoms in optical lattices, we study three different protocols for non-adiabatic quantum state preparation and state transport in chains of Rydberg atoms. The protocols we discuss are based on the blockade mechanism between atoms which, when excited to a Rydberg state, interact through a van der Waals potential, and rely on single-site addressing. Specifically, we discuss protocols for efficient creation of an antiferromagnetic GHZ state, a class of matrix product states including a so-called Rydberg crystal and for the state transport of a single-qubit quantum state between two ends of a chain of atoms. We identify system parameters allowing for the operation of the protocols on timescales shorter than the lifetime of the Rydberg states while yielding high fidelity output states. We discuss the effect of positional disorder on the resulting states and comment on limitations due to other sources of noise such as radiative decay of the Rydberg states. The proposed protocols provide a testbed for benchmarking the performance of quantum information processing platforms based on Rydberg atoms.

Sub-wavelength imaging and field mapping via electromagnetically induced transparency and Autler-Townes splitting in Rydberg atoms

Energy Technology Data Exchange (ETDEWEB)

Holloway, Christopher L., E-mail: holloway@boulder.nist.gov; Gordon, Joshua A. [National Institute of Standards and Technology (NIST), Electromagnetics Division, U.S. Department of Commerce, Boulder Laboratories, Boulder, Colorado 80305 (United States); Schwarzkopf, Andrew; Anderson, David A.; Miller, Stephanie A.; Thaicharoen, Nithiwadee; Raithel, Georg [Department of Physics, University of Michigan, Ann Arbor, Michigan 48109 (United States)

2014-06-16

We present a technique for measuring radio-frequency (RF) electric field strengths with sub-wavelength resolution. We use Rydberg states of rubidium atoms to probe the RF field. The RF field causes an energy splitting of the Rydberg states via the Autler-Townes effect, and we detect the splitting via electromagnetically induced transparency (EIT). We use this technique to measure the electric field distribution inside a glass cylinder with applied RF fields at 17.04 GHz and 104.77 GHz. We achieve a spatial resolution of ≈100 μm, limited by the widths of the laser beams utilized for the EIT spectroscopy. We numerically simulate the fields in the glass cylinder and find good agreement with the measured fields. Our results suggest that this technique could be applied to image fields on a small spatial scale over a large range of frequencies, up into the sub-terahertz regime.

Formation of Antihydrogen Rydberg atoms in strong magnetic field traps

International Nuclear Information System (INIS)

Pohl, T.; Sadeghpour, H. R.

2008-01-01

It is shown that several features of antihydrogen production in nested Penning traps can be described with accurate and efficient Monte Carlo simulations. It is found that cold deeply-bound Rydberg states of antihydrogen (H-bar) are produced in three-body capture in the ATRAP experiments and an additional formation mechanism -Rydberg charge transfer-, particular to the nested Penning trap geometry, is responsible for the observed fast (hot) H-bar atoms. Detailed description of the numerical propagation technique for following extreme close encounters is given. An analytic derivation of the power law behavior of the field ionization spectrum is provided

Experiments with Rydberg atoms on a current-carrying atom chip

NARCIS (Netherlands)

Cisternas San Martín, N.V.

2018-01-01

On one side, atom-chip experiments have demonstrated to be a versatile tool to study quantum physics in cold atoms systems. On the other side, Rydberg atoms have exaggerated properties that makes them good candidates to study quantum information and quantum simulations protocols. In this thesis both

Rubidium-strontium method

International Nuclear Information System (INIS)

Dubansky, A.

1980-01-01

The rubidium-strontium geological dating method is based on the determination of the Rb and Sr isotope ratio in rocks, mainly using mass spectrometry. The method is only practical for silicate minerals and rocks, potassium feldspars and slates. Also described is the rubidium-strontium isochrone method. This, however, requires a significant amount of experimental data and an analysis of large quantities of samples, often of the order of tons. The results are tabulated of rubidium-strontium dating of geological formations in the Czech Socialist Republic. (M.S.)

Rydberg phases of Hydrogen and low energy nuclear reactions

Science.gov (United States)

Olafsson, Sveinn; Holmlid, Leif

2016-03-01

For over the last 26 years the science of cold fusion/LENR has been researched around the world with slow pace of progress. Modest quantity of excess heat and signatures of nuclear transmutation and helium production have been confirmed in experiments and theoretical work has only resulted in a large flora of inadequate theoretical scenarios. Here we review current state of research in Rydberg matter of Hydrogen that is showing strong signature of nuclear processes. In the presentation experimental behavior of Rydberg matter of hydrogen is described. An extensive collaboration effort of surface physics, catalysis, atomic physics, solid state physics, nuclear physics and quantum information is need to tackle the surprising experimental results that have so far been obtained. Rydberg matter of Hydrogen is the only known state of matter that is able to bring huge collection of protons to so short distances and for so long time that tunneling becomes a reasonable process for making low energy nuclear reactions. Nuclear quantum entanglement can also become realistic process at theses conditions.

Optical Measurements of Strong Radio-Frequency Fields Using Rydberg Atoms

Science.gov (United States)

Miller, Stephanie Anne

There has recently been an initiative toward establishing atomic measurement standards for field quantities, including radio-frequency, millimeter-wave, and micro-wave electric fields. Current measurement standards are obtained using dipole antennas, which are fundamentally limited in frequency bandwidth (set by the physical size of the antenna) and accuracy (due to the metal perturbing the field during the measurement). Establishing an atomic standard rectifies these problems. My thesis work contributes to an ongoing effort towards establishing the viability of using Rydberg electromagnetically induced transparency (EIT) to perform atom-based measurements of radio-frequency (RF) fields over a wide range of frequencies and field strengths, focusing on strong-field measurements. Rydberg atoms are atoms with an electron excited to a high principal quantum number, resulting in a high sensitivity to an applied field. A model based on Floquet theory is implemented to accurately describe the observed atomic energy level shifts from which information about the field is extracted. Additionally, the effects due to the different electric field domains within the measurement volume are accurately modeled. Absolute atomic measurements of fields up to 296 V/m within a +/-0.35% relative uncertainty are demonstrated. This is the strongest field measured at the time of data publication. Moreover, the uncertainty is over an order of magnitude better than that of current standards. A vacuum chamber setup that I implemented during my graduate studies is presented and its unique components are detailed. In this chamber, cold-atom samples are generated and Rydberg atoms are optically excited within the ground-state sample. The Rydberg ion detection and imaging procedure are discussed, particularly the high magnification that the system provides. By analyzing the position of the ions, the spatial correlation g(2) (r) of Rydberg-atom distributions can be extracted. Aside from ion

Rydberg Molecules for Ion-Atom Scattering in the Ultracold Regime.

Science.gov (United States)

Schmid, T; Veit, C; Zuber, N; Löw, R; Pfau, T; Tarana, M; Tomza, M

2018-04-13

We propose a novel experimental method to extend the investigation of ion-atom collisions from the so far studied cold, essentially classical regime to the ultracold, quantum regime. The key aspect of this method is the use of Rydberg molecules to initialize the ultracold ion-atom scattering event. We exemplify the proposed method with the lithium ion-atom system, for which we present simulations of how the initial Rydberg molecule wave function, freed by photoionization, evolves in the presence of the ion-atom scattering potential. We predict bounds for the ion-atom scattering length from ab initio calculations of the interaction potential. We demonstrate that, in the predicted bounds, the scattering length can be experimentally determined from the velocity of the scattered wave packet in the case of ^{6}Li^{+}-^{6}Li and from the molecular ion fraction in the case of ^{7}Li^{+}-^{7}Li. The proposed method to utilize Rydberg molecules for ultracold ion-atom scattering, here particularized for the lithium ion-atom system, is readily applicable to other ion-atom systems as well.

Correlations between interacting Rydberg atoms

DEFF Research Database (Denmark)

Paris-Mandoki, Asaf; Braun, Christoph; Hofferberth, Sebastian

2018-01-01

This paper is a short introduction to Rydberg physics and quantum nonlinear optics using Rydberg atoms. It has been prepared as a compliment to a series of lectures delivered during the Latin American School of Physics "Marcos Moshinsky" 2017. We provide a short introduction to the properties...... of individual Rydberg atoms and discuss in detail how the interaction potential between Rydberg atom pairs is calculated. We then discuss how this interaction gives rise to the Rydberg blockade mechanism. With the aid of hallmark experiments in the field applications of the blockade for creating correlated...

Quantum simulation of transverse Ising models with Rydberg atoms

Science.gov (United States)

Schauss, Peter

2018-04-01

Quantum Ising models are canonical models for the study of quantum phase transitions (Sachdev 1999 Quantum Phase Transitions (Cambridge: Cambridge University Press)) and are the underlying concept for many analogue quantum computing and quantum annealing ideas (Tanaka et al Quantum Spin Glasses, Annealing and Computation (Cambridge: Cambridge University Press)). Here we focus on the implementation of finite-range interacting Ising spin models, which are barely tractable numerically. Recent experiments with cold atoms have reached the interaction-dominated regime in quantum Ising magnets via optical coupling of trapped neutral atoms to Rydberg states. This approach allows for the tunability of all relevant terms in an Ising spin Hamiltonian with 1/{r}6 interactions in transverse and longitudinal fields. This review summarizes the recent progress of these implementations in Rydberg lattices with site-resolved detection. Strong correlations in quantum Ising models have been observed in several experiments, starting from a single excitation in the superatom regime up to the point of crystallization. The rapid progress in this field makes spin systems based on Rydberg atoms a promising platform for quantum simulation because of the unmatched flexibility and strength of interactions combined with high control and good isolation from the environment.

Periodically Driven Array of Single Rydberg Atoms

Science.gov (United States)

Basak, Sagarika; Chougale, Yashwant; Nath, Rejish

2018-03-01

An array of single Rydberg atoms driven by a temporally modulated atom-field detuning is studied. The periodic modulation effectively modifies the Rabi coupling, leading to unprecedented dynamics in the presence of Rydberg-Rydberg interactions, in particular, blockade enhancement, antiblockades, and state-dependent population trapping. Interestingly, the Schrieffer-Wolf transformation reveals a fundamental process in Rydberg gases, correlated Rabi coupling, which stems from the extended nature of the Rydberg-Rydberg interactions. Also, the correlated coupling provides an alternative depiction for the Rydberg blockade, exhibiting a nontrivial behavior in the presence of periodic modulation. The dynamical localization of a many-body configuration in a driven Rydberg lattice is discussed.

Motion of Rydberg atoms with strong permanent-electric-dipole interactions

International Nuclear Information System (INIS)

Gonçalves, Luís Felipe; Thaicharoen, Nithiwadee; Raithel, Georg

2016-01-01

Using classical trajectories simulations, we investigate the dynamics of a cold sample of Rydberg atoms with high permanent electric dipole moments. The dipolar state can be created using an adiabatic passage through an avoided crossing between an S-like state and a linear Stark state. The simulations yield the pair-correlation functions (PCF) of the atom samples, which allow us to extract the motion of Rydberg-atom pairs in the many-body system. The results reveal the strength and the anisotropic character of the underlying interaction. The simulation is employed to test the suitability of experimental methods designed to derive interaction parameters from PCF. Insight is obtained about the stability of the method against variation of experimentally relevant parameters. Transient correlations due to interaction-induced heating are observed. (paper)

Janne Rydberg - his life and work

International Nuclear Information System (INIS)

Martinson, I.; Curtis, L.J.

2005-01-01

The Rydberg formula is emblematic of atomic spectroscopy. We review here the personal background, research accomplishments, and academic career of its discoverer, Janne Rydberg. Although his formula is often introduced as a generalization of the hydrogenic Balmer formula, Rydberg's work was independent of Balmer's, and displayed great ingenuity and a rare ability to recognize hidden patterns in complex numerical data. Although his discoveries attracted wide attention, experimental physics was then considered inseparable from measurement, and the fact that Rydberg's insightful formulations used the data of others impeded his academic career. Although Rydberg did not live to see the full theoretical implications of his discoveries, the vigorous study of Rydberg atoms continues today

Accurate values of polarizabilities from Rydberg states

International Nuclear Information System (INIS)

Patil, S.H.

1997-01-01

From the theoretical point of view, there are several properties of Rydberg states which are of interest, interaction of Rydberg atoms with each other, scattering of electrons from Rydberg atoms, interaction of Rydberg atoms with external electromagnetic fields, etc. In this paper the discussion is confined to the particular aspect: the deviations of the energies of Rydberg states from hydrogenic energies, their calculations and their implications from the properties of the core, i.e. the system that remains after Rydberg electron is removed

Correlations between interacting Rydberg atoms

Science.gov (United States)

Paris-Mandoki, Asaf; Braun, Christoph; Hofferberth, Sebastian

2018-04-01

This paper is a short introduction to Rydberg physics and quantum nonlinear optics using Rydberg atoms. It has been prepared as a compliment to a series of lectures delivered during the Latin American School of Physics "Marcos Moshinsky" 2017. We provide a short introduction to the properties of individual Rydberg atoms and discuss in detail how the interaction potential between Rydberg atom pairs is calculated. We then discuss how this interaction gives rise to the Rydberg blockade mechanism. With the aid of hallmark experiments in the field applications of the blockade for creating correlated quantum systems are discussed. Our aim is to give an overview of this exciting and rapidly evolving field. The interested reader is referred to original work and more comprehensive reviews and tutorials for further details on these subjects.

Gauss Sum Factorization with Cold Atoms

International Nuclear Information System (INIS)

Gilowski, M.; Wendrich, T.; Mueller, T.; Ertmer, W.; Rasel, E. M.; Jentsch, Ch.; Schleich, W. P.

2008-01-01

We report the first implementation of a Gauss sum factorization algorithm by an internal state Ramsey interferometer using cold atoms. A sequence of appropriately designed light pulses interacts with an ensemble of cold rubidium atoms. The final population in the involved atomic levels determines a Gauss sum. With this technique we factor the number N=263193

The blue light indicator in rubidium 5S-5P-5D cascade excitation

Science.gov (United States)

Raja, Waseem; Ali, Md. Sabir; Chakrabarti, Alok; Ray, Ayan

2017-07-01

The cascade system has played an important role in contemporary research areas related to fields like Rydberg excitation, four wave mixing and non-classical light generation, etc. Depending on the specific objective, co or counter propagating pump-probe laser experimental geometry is followed. However, the stepwise excitation of atoms to states higher than the first excited state deals with increasingly much fewer number of atoms even compared to the population at first excited level. Hence, one needs a practical indicator to study the complex photon-atom interaction of the cascade system. Here, we experimentally analyze the case of rubidium 5S → 5P → 5D as a specimen of two-step excitation and highlight the efficacy of monitoring one branch, which emits 420 nm, of associated cascade decay route 5D → 6P → 5S, as an effective monitor of the coherence in the system.

Towards the production of an ultra cold antihydrogen beam with the AEGIS apparatus

Energy Technology Data Exchange (ETDEWEB)

Storey, James William, E-mail: james.storey@cern.ch [University of Zurich, Physik-Institut (Switzerland); Collaboration: AEGIS Collaboration

2012-12-15

The AEGIS (Antimatter Experiment: Gravity, Interferometry, Spectroscopy) experiment is an international collaboration, based at CERN, with the experimental goal of performing the first direct measurement of the Earth's gravitational acceleration on antihydrogen. In the first phase of the experiment, a gravity measurement with 1% precision will be performed by passing a beam of ultra cold antihydrogen atoms through a classical Moire deflectometer coupled to a position sensitive detector. The key requirements for this measurement are the production of ultra cold (T{approx}100 mK) Rydberg state antihydrogen and the subsequent Stark acceleration of these atoms. The aim is to produce Rydberg state antihydrogen by means of the charge exchange reaction between ultra cold antiprotons (T{approx}100 mK) and Rydberg state positronium. This paper will present details of the developments necessary for the successful production of the ultra cold antihydrogen beam, with emphasis on the detector that is required for the development of these techniques. Issues covered will include the detection of antihydrogen production and temperature, as well as detection of the effects of Stark acceleration.

Generation and storage of quantum states using cold atoms

DEFF Research Database (Denmark)

Dantan, Aurelien Romain; Josse, Vincent; Cviklinski, Jean

2006-01-01

Cold cesium or rubidium atomic samples have a good potential both for generation and storage of nonclassical states of light. Generation of nonclassical states of light is possible through the high non-linearity of cold atomic samples excited close to a resonance line. Quadrature squeezing, polar...

Collisional destruction of fast hydrogen Rydberg atoms

International Nuclear Information System (INIS)

King, M.R.

1984-01-01

A new modulated electric field technique was developed to study Rydberg atom destruction processes in a fast beam. The process of destruction of a band of Rydberg atom destruction of a band of Rydberg atoms through the combined processes of ionization, excitation, and deexcitation was studied for collisions with gas targets. Rydberg atoms of hydrogen were formed by electron capture, and detected by field ionization. The modulated field technique described proved to be an effective technique for producing a large signal for accurate cross section measurements. The independent particle model for Rydberg atom destruction processes was found to hold well for collisions with molecular nitrogen, argon, and carbon dioxide. The resonances in the cross sections for the free electron scattering with these targets were found to also occur in Rydberg destruction. Suggestions for future investigations of Rydberg atom collision processes in the fast beam regime are given

A high resolution ion microscope for cold atoms

International Nuclear Information System (INIS)

Stecker, Markus; Schefzyk, Hannah; Fortágh, József; Günther, Andreas

2017-01-01

We report on an ion-optical system that serves as a microscope for ultracold ground state and Rydberg atoms. The system is designed to achieve a magnification of up to 1000 and a spatial resolution in the 100 nm range, thereby surpassing many standard imaging techniques for cold atoms. The microscope consists of four electrostatic lenses and a microchannel plate in conjunction with a delay line detector in order to achieve single particle sensitivity with high temporal and spatial resolution. We describe the design process of the microscope including ion-optical simulations of the imaging system and characterize aberrations and the resolution limit. Furthermore, we present the experimental realization of the microscope in a cold atom setup and investigate its performance by patterned ionization with a structure size down to 2.7 μ m. The microscope meets the requirements for studying various many-body effects, ranging from correlations in cold quantum gases up to Rydberg molecule formation. (paper)

Bohmian picture of Rydberg atoms

Indian Academy of Sciences (India)

Abstract. Unlike the previous theoretical results based on standard quantum mechanics that established the nearly elliptical shapes for the centre-of-mass motion in Rydberg atoms using numerical simulations, we show analytically that the Bohmian trajectories in Rydberg atoms are nearly elliptical.

Myocardial study with rubidium-82 using positron emission tomography

Energy Technology Data Exchange (ETDEWEB)

De Landsheere, C.; Brihaye, C.; Chevigne, M.; Guillaume, M.; Lamotte, D.; Larock, M.P.; Quaglia, L.; Rigo, P. (Universite de Liege (Belgium))

1982-01-01

The rubidium-82 is eluted from a strontium-82/rubidium-82 generator. Its short half-life (78 sec.) enables the sequential repetition of dynamic studies. Myocardial ischemia produced in the dog by a stenosis of the left anterior descending artery is investigated. In this case, intravenous administration of rubidium demonstrates a decrease in the cation uptake in the anterior wall of the left ventricle. Through ischemia studies various parameters which are liked to modify the rubidium distribution according to the equation describing the cation exchanges, are considered. The generator strontium-82/rubidium-82 delivers a reference tracer for myocardial flow evaluation without requiring a cyclotron which is then available for the direct production of metabolic tracers.

Electromagnetically Induced Transparency In Rydberg Atomic Medium

Science.gov (United States)

Deng, Li; Cong, Lu; Chen, Ai-Xi

2018-03-01

Due to possessing big principal quantum number, Rydberg atom has some unique properties, for example: its radiative lifetime is long, dipole moment is large, and interaction between atoms is strong and so on. These properties make one pay attention to Rydberg atoms. In this paper we investigate the effects of Rydberg dipole-dipole interactions on electromagnetically induced transparency (EIT) schemes and group velocity in three-level systems of ladder type, which provides theoretical foundation for exploring the linear and nonlinear characteristics of light in a Rydberg electromagnetically-induced-transparency medium.

Calculation of Rydberg interaction potentials

International Nuclear Information System (INIS)

Weber, Sebastian; Büchler, Hans Peter; Tresp, Christoph; Urvoy, Alban; Hofferberth, Sebastian; Menke, Henri; Firstenberg, Ofer

2017-01-01

The strong interaction between individual Rydberg atoms provides a powerful tool exploited in an ever-growing range of applications in quantum information science, quantum simulation and ultracold chemistry. One hallmark of the Rydberg interaction is that both its strength and angular dependence can be fine-tuned with great flexibility by choosing appropriate Rydberg states and applying external electric and magnetic fields. More and more experiments are probing this interaction at short atomic distances or with such high precision that perturbative calculations as well as restrictions to the leading dipole–dipole interaction term are no longer sufficient. In this tutorial, we review all relevant aspects of the full calculation of Rydberg interaction potentials. We discuss the derivation of the interaction Hamiltonian from the electrostatic multipole expansion, numerical and analytical methods for calculating the required electric multipole moments and the inclusion of electromagnetic fields with arbitrary direction. We focus specifically on symmetry arguments and selection rules, which greatly reduce the size of the Hamiltonian matrix, enabling the direct diagonalization of the Hamiltonian up to higher multipole orders on a desktop computer. Finally, we present example calculations showing the relevance of the full interaction calculation to current experiments. Our software for calculating Rydberg potentials including all features discussed in this tutorial is available as open source. (tutorial)

Sympathetic cooling in a rubidium cesium mixture: Production of ultracold cesium atoms; Sympathetisches Kuehlen in einer Rubidium-Caesium-Mischung: Erzeugung ultrakalter Caesiumatome

Energy Technology Data Exchange (ETDEWEB)

Haas, M.

2007-07-01

This thesis presents experiments for the production of ultracold rubidium cesium mixture in a magnetic trap. The long-termed aim of the experiment is the study of the interaction of few cesium atoms with a Bose-Einstein condensate of rubidium atoms. Especially by controlled variation of the cesium atom number the transition in the description of the interaction by concepts of the one-particle physics to the description by concepts of the many-particle physics shall be studied. The rubidium atoms are trapped in a magneto-optical trap (MOT) and from there reloaded into a magnetic trap. In this the rubidium atoms are stored in the state vertical stroke f=2,m{sub f}=2 right angle of the electronic ground state and evaporatively cooled by means of microwave-induced transitions into the state vertical stroke f=1,m{sub f}=1] (microwave cooling). The cesium atoms are also trppaed in a MOT and into the same magnetic trap reloaded, in which they are stored in the state vertical stroke f=4,m{sub f}=4 right angle of the electronic ground state together with rubidium. Because of the different hyperfine splitting only rubidium is evaporatively cooled, while cesium is cooled jointly sympathetically - i.e. by theramal contact via elastic collisions with rubidium atoms. The first two chapters contain a description of interatomic interactions in ultracold gases as well as a short summary of theoretical concepts in the description of Bose-Einstein condensates. The chapters 3 and 4 contain a short presentation of the methods applied in the experiment for the production of ultracold gases as well as the experimental arrangement; especially in the framework of this thesis a new coil system has been designed, which offers in view of future experiments additionally optical access for an optical trap. Additionally the fourth chapter contains an extensive description of the experimental cycle, which is applied in order to store rubidium and cesium atoms together into the magnetic trap. The

Magnetic trapping of Rydberg atoms

NARCIS (Netherlands)

Niestadt, D.; Naber, J.; Kokkelmans, S.J.J.M.F.; Spreeuw, R.J.C.

2016-01-01

Magnetic trapping is a well-established technique for ground state atoms. We seek to extend this concept to Rydberg atoms. Rydberg atoms are important for current visions of quantum simulators that will be used in the near future to simulate and analyse quantum problems. Current efforts in Amsterdam

Development of rubidium and niobium containing plastic foams. Final report

International Nuclear Information System (INIS)

Botham, R.A.; McClung, C.E.; Schwendeman, J.I.

1978-01-01

Rubidium fluoride and niobium metal-containing foam samples (rods and sheets) were prepared using two foam sytems: (1) hydrophilic polyurethanes prepared from W.R. Grace Co.'s Hypol prepolymers and (2) polyimides prepared from Monsanto Company's Skybond polyimide resin. The first system was used only for preparation of rubidium fluoride-containing foams while the second was used for both rubidium fluoride and niobium-containing foams. The niobium metal could readily be incorporated into the polyimide foam during molding, to produce foam sheets of the required dimensions and density. The rubidium fluoride-containing polyimide foams were preferably prepared by first rendering the molded polyimide foam hydrophilic with a postcuring treatment, then absorbing the rubidium fluoride from water solution. Similarly, rubidium fluoride was absorbed into the hydrophilic polyurethanes from water solution. Since the high reactive rubidium metal could not be employed, rubidium fluoride, which is very hygroscopic, was used instead, primarily because of its high rubidium content (approximately 82 weight percent). This was important in view of the low total densities and the high weight percentage rubidium required in the foam samples. In addition, at the later request of LLL, a block of rigid Hypol hydrophilic polyurethane foam (with a density of approximately 0.04 g/cm 3 and cell sizes = or <0.2 mm) was prepared without any metal or metal compounds in it. Two shipments of foam samples, which met or closely approximated the project specifications, were submitted to LLL during the course of this project. Information on these samples is contained in Table 1. A complete description of their preparation is given in the Experimental Results and Discussion Section

Trapping of Rydberg atoms in tight magnetic microtraps

NARCIS (Netherlands)

Boetes, A.Q.G.; Skannrup, R.V.; Naber, J.; Kokkelmans, S.J.J.M.F.; Spreeuw, R.J.C.

2018-01-01

We explore the possibility to trap Rydberg atoms in tightly confining magnetic microtraps. The trapping frequencies for Rydberg atoms are expected to be influenced strongly by magnetic-field gradients. We show that there are regimes where Rydberg atoms can be trapped. Moreover, we show that

Surface Plasmon Polaritons Probed with Cold Atoms

DEFF Research Database (Denmark)

Kawalec, Tomasz; Sierant, Aleksandra; Panas, Roman

2017-01-01

We report on an optical mirror for cold rubidium atoms based on a repulsive dipole potential created by means of a modified recordable digital versatile disc. Using the mirror, we have determined the absolute value of the surface plasmon polariton (SPP) intensity, reaching 90 times the intensity...

"Chemical contraction" in rubidium-bismuth melts

Science.gov (United States)

Khairulin, R. A.; Abdullaev, R. N.; Stankus, S. V.

2017-10-01

The density and thermal expansion of liquid rubidium and rubidium-bismuth alloy containing 25.0 at % Bi were measured by the gamma-ray attenuation technique at temperatures from liquidus to 1000 K. The results of this study were compared with the data obtained by other authors. The molar volume of the Rb75Bi25 melt strongly deviates from the additivity rule for ideal solutions.

Intracoronary use of rubidium-82

International Nuclear Information System (INIS)

Harper, P.V.; Ryan, J.W.; Al-Sadir, J.; Chua, K.G.; Resnekov, L.; Nierinckx, R.; Loberg, M.

1985-01-01

Rubidium-82 (75 sec) is well suited for myocardial localization studies performed by intracoronary injection in connection with coronary angiography. Rubidium ion is efficiently extracted from the blood so that blood background and radiation to other organs such as the kidneys are greatly reduced, as is the amount of activity required to make satisfactory images. Pilot studies in 15 patients have resulted in no complications. Feasibility has been demonstrated for pacing studies and for drug intervention with nitroglycerine. Uptake defects correlate well with vascular lesions

One-Dimensional Rydberg Gas in a Magnetoelectric Trap

International Nuclear Information System (INIS)

Mayle, Michael; Hezel, Bernd; Lesanovsky, Igor; Schmelcher, Peter

2007-01-01

We study the quantum properties of Rydberg atoms in a magnetic Ioffe-Pritchard trap which is superimposed by a homogeneous electric field. Trapped Rydberg atoms can be created in long-lived electronic states exhibiting a permanent electric dipole moment of several hundred Debye. The resulting dipole-dipole interaction in conjunction with the radial confinement is demonstrated to give rise to an effectively one-dimensional ultracold Rydberg gas with a macroscopic interparticle distance. We derive analytical expressions for the electric dipole moment and the required linear density of Rydberg atoms

Dual cesium and rubidium atomic fountain with a 10-16 level accuracy and applications

International Nuclear Information System (INIS)

Chapelet, F.

2008-05-01

Atomic fountains are the most accomplished development of the atomic clocks based on the cesium atom whose hyperfine resonance defines the SI second since 1967. Today these systems are among those which realize the second with the best accuracy. We present the last developments of the cold cesium and rubidium atom dual fountain experiment at LNE-SYRTE. This unique dual setup would allow to obtain an outstanding resolution in fundamental physics tests based on atomic transition frequency comparisons. In order to enable operation with both atomic species simultaneously, we designed, tested and implemented on the fountain new collimators which combine the laser lights corresponding to each atom. By comparing our rubidium fountain to another cesium fountain over a decade, we performed a test of the stability of the fine structure constant at the level of 5 * 10 -16 per year. We carried on the work on the clock accuracy and we focused on the phase gradients effects in the interrogation cavity and on the microwave leakage. The fountain accuracy has been evaluated to 4 * 10 -16 for the cesium clock and to 5 * 10 -16 for the refurbished rubidium clock. As a powerful instrument of metrology, our fountain was implicated in many clock comparisons and contributed many times to calibrate the International Atomic Time. Furthermore, we used the fountain to perform a new test of Lorentz local invariance. (author)

Cardiac 82rubidium PET/CT: initial European experience

International Nuclear Information System (INIS)

Groves, Ashley M.; Dickson, John C.; Kayani, Irfan; Endozo, Raymondo; Blanchard, Patty; Shastry, Manu; Prvulovich, Elizabeth; Waddington, Wendy A.; Ben-Haim, Simona; Bomanji, Jamshed B.; Ell, Peter J.; Speechly-Dick, Marie-Elsya; McEwan, Jean R.

2007-01-01

Myocardial perfusion with PET/CT has advantages over conventional SPECT. We describe our initial European experience using 82 Rubidium-PET/CT, as part of a clinical myocardial perfusion service. We studied the first 100 patients (64 male; 36 female, mean age = 60: SD +/-12.5y, mean body mass index = 30: SD +/-6.9kg/m 2 ) who underwent 82 Rubidium cardiac PET/CT in our institution. Thirty patients had recently undergone coronary angiography. Patients underwent imaging during adenosine infusion and at rest. Images were acquired over 5 minutes using a GE-PET/CT instrument. Image quality was described as good, adequate or inadequate. Images were reported patient-by-patient by a minimum of five nuclear medicine physicians. A segment-by-segment analysis (17-segment model) was also performed. Image quality was good in 77%, adequate 23% and inadequate 0%. There was no statistical difference in image quality between obese and non-obese patients (Fisher's exact test, p = 0.2864). 59% had normal perfusion studies, 29% had inducible ischaemia, 12% had myocardial infarction (11% with super added ischaemia). There was reduced 82 Rubidium uptake in 132/1700 segments during stress. There was reduced 82 Rubidium uptake at rest in 42/1700 segments. The 82 Rubidium PET/CT findings were consistent with the angiographic findings in 28/30 cases. We show that, even from initial use of 82 Rubidium, it is possible to perform myocardial perfusion studies quickly with good image quality, even in the obese. The PET findings correlated well in the third of the cases where angiography was available. As such, 82 Rubidium cardiac PET/CT is likely to be an exciting addition to the European nuclear physician/ cardiologist's radionuclide imaging arsenal. (orig.)

Correlated Photon Dynamics in Dissipative Rydberg Media

Science.gov (United States)

Zeuthen, Emil; Gullans, Michael J.; Maghrebi, Mohammad F.; Gorshkov, Alexey V.

2017-07-01

Rydberg blockade physics in optically dense atomic media under the conditions of electromagnetically induced transparency (EIT) leads to strong dissipative interactions between single photons. We introduce a new approach to analyzing this challenging many-body problem in the limit of a large optical depth per blockade radius. In our approach, we separate the single-polariton EIT physics from Rydberg-Rydberg interactions in a serialized manner while using a hard-sphere model for the latter, thus capturing the dualistic particle-wave nature of light as it manifests itself in dissipative Rydberg-EIT media. Using this approach, we analyze the saturation behavior of the transmission through one-dimensional Rydberg-EIT media in the regime of nonperturbative dissipative interactions relevant to current experiments. Our model is able to capture the many-body dynamics of bright, coherent pulses through these strongly interacting media. We compare our model with available experimental data in this regime and find good agreement. We also analyze a scheme for generating regular trains of single photons from continuous-wave input and derive its scaling behavior in the presence of imperfect single-photon EIT.

Two electron Rydberg states

International Nuclear Information System (INIS)

Cooke, W.E.

1981-01-01

This paper addresses the study of two-electron Rydberg atoms. With Multichannel Quantum Defect Theory (MQDT), there is a technique for characterizing a spectra in terms of a small number of parameters. A survey of some important effects specific to two-electon Rydberg states, using primarily the alkaline earth atoms for examples, is made. The remainder of the paper deals with a discussion of the electron-electron interaction, including some of the basic points of MQDT. Energy exchange between two electrons is also addressed

n l -> n' l' transition rates in electron and proton - Rydberg atom collision

Science.gov (United States)

Vrinceanu, Daniel

2017-04-01

Electrons and protons drive the recombination dynamics of highly excited Rydberg atoms in cold rarefied plasmas found in astrophysical conditions such as primordial recombination or star formation in H-II clouds. It has been recognized that collisions induce both energy and angular momentum transitions in Rydberg atoms, although in different proportions, depending on the initial state, temperature and the given species considered in the collision (electron or proton). Most studies focused on one collision type at a time, under the assumption that collision types are independent or their effects are not competing. The classical Monte-Carlo trajectory simulations presented in this work calculate the rates for both energy and angular momentum transfers and show their interdependence. For example, energy transfer with small angular momentum change are more efficient for target states with initial large angular momentum. The author acknowledges support received from the National Science Foundation through a Grant for the Center for Research on Complex Networks (HRD-1137732).

Electromagnetically induced transparency of ultra-long-range Rydberg molecules

DEFF Research Database (Denmark)

Mirgorodskiy, Ivan; Christaller, Florian; Braun, Christoph

2017-01-01

We study the impact of Rydberg molecule formation on the storage and retrieval of Rydberg polaritons in an ultracold atomic medium. We observe coherent revivals appearing in the storage and retrieval efficiency of stored photons that originate from simultaneous excitation of Rydberg atoms and Ryd...

Verification of rubidium-82 for heart studies

International Nuclear Information System (INIS)

Budinger, T.F.; Yano, Y.; Twitchell, J.A.; Brennan, K.M.

1985-01-01

Whereas 82 Rb has been shown to reflect heart blood-flow under normal circumstances and has the great benefit of being available from a noncyclotron source, there remains a question with regard to the physiology of rubidium transport into the heart muscle. The fraction of the amount of the rubidium tracer that goes into the heart varies with flow, and, unfortunately, the amount that accumulates in the muscle will not therefore be proportional to flow. Over the past three years, the authors have re-evaluated this question and determined that the uptake of rubidium in the myocardium follows a simple model of conservation of mass wherein the amount that is present is equal to the product of flow times extraction

Dual cesium and rubidium atomic fountain with a 10{sup -16} level accuracy and applications; Fontaine atomique double de cesium et de rubidium avec une exactitude de quelques 10{sup -16} et applications

Energy Technology Data Exchange (ETDEWEB)

Chapelet, F

2008-05-15

Atomic fountains are the most accomplished development of the atomic clocks based on the cesium atom whose hyperfine resonance defines the SI second since 1967. Today these systems are among those which realize the second with the best accuracy. We present the last developments of the cold cesium and rubidium atom dual fountain experiment at LNE-SYRTE. This unique dual setup would allow to obtain an outstanding resolution in fundamental physics tests based on atomic transition frequency comparisons. In order to enable operation with both atomic species simultaneously, we designed, tested and implemented on the fountain new collimators which combine the laser lights corresponding to each atom. By comparing our rubidium fountain to another cesium fountain over a decade, we performed a test of the stability of the fine structure constant at the level of 5 * 10{sup -16} per year. We carried on the work on the clock accuracy and we focused on the phase gradients effects in the interrogation cavity and on the microwave leakage. The fountain accuracy has been evaluated to 4 * 10{sup -16} for the cesium clock and to 5 * 10{sup -16} for the refurbished rubidium clock. As a powerful instrument of metrology, our fountain was implicated in many clock comparisons and contributed many times to calibrate the International Atomic Time. Furthermore, we used the fountain to perform a new test of Lorentz local invariance. (author)

revivals of Rydberg wave packets

International Nuclear Information System (INIS)

Bluhm, R.; Kostelecky, V.A.; Tudose, B.

1998-01-01

We examine the revival structure of Rydberg wave packets. The effects of quantum defects on wave packets in alkali-metal atoms and a squeezed-state description of the initial wave packets are also described. We then examine the revival structure of Rydberg wave packets in the presence of an external electric field, i.e., the revival structure of Stark wave packets. These wave packets have energies that depend on two quantum numbers and exhibit new types of interference behaviour

Stress/Rest Tc-99m-MIBI SPECT in Comparison with Rest/Stress Rubidium - 82 PET

International Nuclear Information System (INIS)

Lee, D. S.; Kamg, K. W.; Lee, K. H.; Jeong, J. M.; Kwark, C. E.; Chung, J. K.; Lee, M.C.; Seo, J. D.; Koh, C. S.

1995-01-01

We compared stress/rest myocardial Tc-99m-MIBI tomographic image findings with rest/stress rubidium-82 tomographic images. In 23 patients with coronary artery disease (12 of them received bypass grafts before) and 6 normal subjects, rest rubidium PET study was performed, rubidium-82 and Tc-99m-MIBI were injected simultaneously to each patient after dipyridamole stress for rubidium PET and MIBI SPECT; and rest MIBI SPECT was performed 4 hours thereafter. We scored segmental decrease of rubidium, or MIBI uptakes into 5 grades for 29 segments from 3 short-axis, vertical and horizontal slices. Scores were summed for each major arterial territory. When more score than two grade-2's or one grade-3 was considered as the cue for significant stenosis for major arterial territories, 67% of 46 stenosed arteries were found with MIBI studies and 78% of them by rubidium studies. Fourteen among 28 grafted arterial territories of 12 post-CABG patients were found normal with both rubidium and MIBI. Segmental scores were concordant between rubidium and MIBI in 72% of 709-stress segments and in 80% of 825 rest segments. Stress rubidium segmental scores were less than stress MIBI scores in 9%, so were rest rubidium scores. Stress rubidium scores were more than stress MIBI scores in 20% of segments, and rest rubidium segmental scores were more than rest MIBI scores in 11%. Rank correlations (Spearman's rho's more than 0.7(stress) and 0.5(rest), slopes (MIBI/rubidium) around 0.7(stress) and 0.9(rest) suggested deeper and wider defects in stress with rubidium. Slope over 1 (MIBI/rubidium) with LAD segmental scores at rest and 7 territories which had much larger score with MIBI revealed exaggeration of rest defects with rest MIBI in same-day stress/rest study. Difference scores (stress-rest for each territory) suggesting ischemia were larger with rubidium (slope of MIBI/rubidium around 0.45). As has been implied by animal or separate-day- human studies, these segmental analyses with

Determination of lithium, rubidium and strontium in foodstuffs

International Nuclear Information System (INIS)

Evans, W.H.; Read, J.I.

1985-01-01

For the determination of total lithium, rubidium and strontium in foodstuffs the organic matter is destroyed by a wet-oxidation procedure. Both lithium and rubidium are measured by flame atomic-emission spectrophotometry, rubidium with the addition of a radiation buffer and strontium is measured by flame atomic-absorption spectrophotometry using the same radiation buffer. The optimum conditions for measurement are described and interferences noted. The accuracy of the method was assessed by measuring the recovery of these metals from foodstuff homogenates and values for standard reference materials are listed, for comparison with certified levels where these exist. From the results obtained standard deviations were calculated and derived limits of detection and confidence intervals are given. (author)

Separation of rubidium from irradiated aluminum-encapsulated uranium

International Nuclear Information System (INIS)

Horwitz, E.P.; Schmitz, F.J.; Rokop, D.J.

1982-01-01

A procedure was developed for separating rubidium from irradiated aluminum encapsulated uranium. The separations procedure produces a final ultra-high purity RbCl product for subsequent high performance mass spectrometric analysis. The procedure involves first removing most of the macro-components and fission products by strong base anion exchange using, first, concentrated HCl, then oxalic acid media and second, selectively separating rubidium from alkaline-earth ions and other alkali-metal ions, including cesium, using Bio-Rex-40 cation-exchange resin. The resultant RbCl is then put through a final vacuum sublimation step. Ultra-pure reagents and specially clean glassware are used throughout the procedure to minimize contamination by naturally-occurring rubidium

Many-body physics with alkaline-earth Rydberg lattices

Energy Technology Data Exchange (ETDEWEB)

Mukherjee, R; Nath, R; Pohl, T [Max Planck Institute for the Physics of Complex Systems, Noethnitzer Strasse 38, 01187 Dresden (Germany); Millen, J; Jones, M P A, E-mail: rick@pks.mpg.de [Department of Physics, Durham University, Durham DH1 3LE (United Kingdom)

2011-09-28

We explore the prospects for confining alkaline-earth Rydberg atoms in an optical lattice via optical dressing of the secondary core-valence electron. Focussing on the particular case of strontium, we identify experimentally accessible magic wavelengths for simultaneous trapping of ground and Rydberg states. A detailed analysis of relevant loss mechanisms shows that the overall lifetime of such a system is limited only by the spontaneous decay of the Rydberg state, and is not significantly affected by photoionization or autoionization. The van der Waals C{sub 6} coefficients for the Sr(5sns {sup 1}S{sub 0}) Rydberg series are calculated, and we find that the interactions are attractive. Finally we show that the combination of magic-wavelength lattices and attractive interactions could be exploited to generate many-body Greenberger-Horne-Zeilinger states.

Calculation of Rydberg interaction potentials

DEFF Research Database (Denmark)

Weber, Sebastian; Tresp, Christoph; Menke, Henri

2017-01-01

The strong interaction between individual Rydberg atoms provides a powerful tool exploited in an ever-growing range of applications in quantum information science, quantum simulation and ultracold chemistry. One hallmark of the Rydberg interaction is that both its strength and angular dependence...... for calculating the required electric multipole moments and the inclusion of electromagnetic fields with arbitrary direction. We focus specifically on symmetry arguments and selection rules, which greatly reduce the size of the Hamiltonian matrix, enabling the direct diagonalization of the Hamiltonian up...

Sympathetic cooling in a rubidium cesium mixture: Production of ultracold cesium atoms

International Nuclear Information System (INIS)

Haas, M.

2007-01-01

This thesis presents experiments for the production of ultracold rubidium cesium mixture in a magnetic trap. The long-termed aim of the experiment is the study of the interaction of few cesium atoms with a Bose-Einstein condensate of rubidium atoms. Especially by controlled variation of the cesium atom number the transition in the description of the interaction by concepts of the one-particle physics to the description by concepts of the many-particle physics shall be studied. The rubidium atoms are trapped in a magneto-optical trap (MOT) and from there reloaded into a magnetic trap. In this the rubidium atoms are stored in the state vertical stroke f=2,m f =2 right angle of the electronic ground state and evaporatively cooled by means of microwave-induced transitions into the state vertical stroke f=1,m f =1] (microwave cooling). The cesium atoms are also trppaed in a MOT and into the same magnetic trap reloaded, in which they are stored in the state vertical stroke f=4,m f =4 right angle of the electronic ground state together with rubidium. Because of the different hyperfine splitting only rubidium is evaporatively cooled, while cesium is cooled jointly sympathetically - i.e. by theramal contact via elastic collisions with rubidium atoms. The first two chapters contain a description of interatomic interactions in ultracold gases as well as a short summary of theoretical concepts in the description of Bose-Einstein condensates. The chapters 3 and 4 contain a short presentation of the methods applied in the experiment for the production of ultracold gases as well as the experimental arrangement; especially in the framework of this thesis a new coil system has been designed, which offers in view of future experiments additionally optical access for an optical trap. Additionally the fourth chapter contains an extensive description of the experimental cycle, which is applied in order to store rubidium and cesium atoms together into the magnetic trap. The last chapter

Improvement on Temperature Measurement of Cold Atoms in a Rubidium Fountain

International Nuclear Information System (INIS)

Lü De-Sheng; Qu Qiu-Zhi; Wang Bin; Zhao Jian-Bo; Liu Liang; Wang Yu-Zhu

2011-01-01

The time-of-flight (TOF) method is one of the most common ways to measure the temperature of cold atoms. In the cold atomic fountain setup, the geometry of the probe beam will introduce the measurement errors to the spatial distribution of cold atomic cloud, which will lead to the measurement errors on atomic temperature. Using deconvolution, we recover the atomic cloud profile from the TOF signal. Then, we use the recovered signals other than the TOF signals to obtain a more accurate atomic temperature. This will be important in estimating the effects of cold atom collision shift and the shift due to transverse cavity phase distribution on an atomic fountain clock. (atomic and molecular physics)

Substoichiometric extraction of rubidium with Dibenzo-24-crown-8 into Xylene

International Nuclear Information System (INIS)

Bag, M.; Chattopadhyay, P.; Basu, S.

2014-01-01

Owing to immense applications of rubidium in varied fields, extraction and quantification of rubidium have gained great importance in recent years. Here, studies on substoichiometric extraction of rubidium by dibenzo-24-crown-8 into xylene using 86 Rb radiotracer are reported. The method has been optimized by pH of the medium, effects of diverse ions, etc, to explore its applicability in real samples

Addendum to ''Density fluctuations in liquid rubidium''

International Nuclear Information System (INIS)

Haan, S.W.; Mountain, R.D.; Hsu, C.S.; Rahman, A.

1980-01-01

We performed molecular-dynamics simulations of liquid rubidium and the Lennard-Jones fluid at several densities and temperatures, and of a system whose pair potential is the repulsive core of the rubidium potential. In all cases, propagating density fluctuations occurred in the rubidiumlike systems at much shorter wavelengths than in the Lennard-Jones system. This indicates that the repulsive part of the pair potential is the dominant factor in determining the relaxation of short-wavelength density fluctuations

Stage structure and electrical properties of rubidium-doped pentacene

International Nuclear Information System (INIS)

Matsuo, Yasumitsu; Sasaki, Sachio; Ikehata, Seiichiro

2004-01-01

We have investigated the structural and electrical properties on the molecular conductor based on pentacene doped with rubidium. It was found from the X-ray diffraction measurement that the rubidium-doped pentacene becomes a highly oriented film with a stage-1 structure, as seen in graphite intercalated compounds. It was also found from this result that the length between pentacene molecular layers increases from 1.51 nm of pure pentacene to 1.62 nm. Moreover, the result of the electrical conductivity measurement shows that by doping of rubidium electrical conductivity at room temperature increases above 10 8 times larger than that of pure pentacene. We have also found that the electrical conductivity along the a-b plane (parallel to the molecular layers) is 10 2 times larger than that along the c-axis which is perpendicular to the molecular layers. These results indicate that pentacene doped with rubidium becomes a molecular conductor and displays the quasi-two-dimensional conductivity

Rydberg atoms in strong fields

International Nuclear Information System (INIS)

Kleppner, D.; Tsimmerman, M.

1985-01-01

Experimental and theoretical achievements in studying Rydberg atoms in external fields are considered. Only static (or quasistatic) fields and ''one-electron'' atoms, i.e. atoms that are well described by one-electron states, are discussed. Mainly behaviour of alkali metal atoms in electric field is considered. The state of theoretical investigations for hydrogen atom in magnetic field is described, but experimental data for atoms of alkali metals are presented as an illustration. Results of the latest experimental and theoretical investigations into the structure of Rydberg atoms in strong fields are presented

Quantum information with Rydberg atoms

DEFF Research Database (Denmark)

Saffman, Mark; Walker, T.G.; Mølmer, Klaus

2010-01-01

Rydberg atoms with principal quantum number n»1 have exaggerated atomic properties including dipole-dipole interactions that scale as n4 and radiative lifetimes that scale as n3. It was proposed a decade ago to take advantage of these properties to implement quantum gates between neutral atom...... of multiqubit registers, implementation of robust light-atom quantum interfaces, and the potential for simulating quantum many-body physics. The advances of the last decade are reviewed, covering both theoretical and experimental aspects of Rydberg-mediated quantum information processing....

Spectrum of spin waves in cold polarized gases

Energy Technology Data Exchange (ETDEWEB)

Andreeva, T. L., E-mail: phdocandreeva@yandex.ru [Russian Academy of Sciences, Lebedev Physical Institute (Russian Federation)

2017-02-15

The spin dynamics of cold polarized gases are investigated using the Boltzmann equation. The dispersion relation for spin waves (transverse component of the magnetic moment) and the spin diffusion coefficient of the longitudinal component of the magnetic moment are calculated without using fitting parameters. The spin wave frequency and the diffusion coefficient for rubidium atoms are estimated numerically.

Ionization due to the interaction between two Rydberg atoms

International Nuclear Information System (INIS)

Robicheaux, F

2005-01-01

Using a classical trajectory Monte Carlo method, we have computed the ionization resulting from the interaction between two cold Rydberg atoms. We focus on the products resulting from close interaction between two highly excited atoms. We give information on the distribution of ejected electron energies, the distribution of internal atom energies and the velocity distribution of the atoms and ions after the ionization. If the potential for the atom is not purely Coulombic, the average interaction between two atoms can change from attractive to repulsive giving a Van de Graaff-like mechanism for accelerating atoms. In a small fraction of ionization cases, we find that the ionization leads to a positive molecular ion where all of the distances are larger than 1000 Bohr radii

Coopetition and manipulation of quantum correlations in Rydberg atoms

International Nuclear Information System (INIS)

Fan, Chu-Hui; Yan, Dong; Liu, Yi-Mou; Wu, Jin-Hui

2017-01-01

We study the steady-state quantum correlations arising from the atom–field and interatomic interplays in two-level Rydberg atoms coherently driven by an external laser field. Three kinds of quantum correlations, i.e., atom–atom correlation, atom–field entanglement and photon–photon correlation, are simultaneously examined by considering dipole–dipole interactions (DDI) for pairwise Rydberg atoms. They are shown to be closely linked with single and double Rydberg excitations, which can be modulated to work in the blockade or antiblockade regime depending on the driving field frequency, the DDI strength and the Rydberg decay rate. As a result, we obtain strongly correlated atoms and highly antibunching photons (indispensable resources in applications of quantum information processing) intermediated with robust atom–field entanglement. (paper)

Jahn-Teller effect in Rydberg series: A multi-state vibronic coupling problem

International Nuclear Information System (INIS)

Staib, A.; Domcke, W.; Sobolewski, A.L.

1990-01-01

Two simple limiting cases of Jahn-Teller (JT) coupling in Rydberg states of polyatomic molecules are considered, namely (i) JT coupling in Rydberg orbitals as well as in the ionization continuum (nondegenerate ion core, degenerate Rydberg series) and (ii) JT coupling in the ion core (degenerate ion core, nondegenerate Rydberg series). For both models simple and efficient algorithms for the computation of spectra (dynamical JT effect) are developed. The orbital JT effect is shown to represent a novel type of multi-state vibronic coupling, giving rise to interesting spectroscopic phenomena, among them resonant inter-Rydberg perturbations and JT induced autoionization. Particular attention is paid to the demonstration of the characteristic spectroscopic signatures of the two types of JT coupling in Rydberg states. (orig.)

Rydberg-Stark states of Positronium for atom optics

International Nuclear Information System (INIS)

Alonso, A M; Cooper, B S; Deller, A; Hogan, S D; Wall, T E; Cassidy, D B

2015-01-01

Positronium atoms were produced in Rydberg states by means of a two-step optical excitation process (1s→2p→nd/ns). The n = 11 Rydberg-Stark manifold has been studied using different laser polarizations providing greater control over the electric dipole moment. (paper)

Theory of long-range interactions for Rydberg states attached to hyperfine-split cores

Science.gov (United States)

Robicheaux, F.; Booth, D. W.; Saffman, M.

2018-02-01

The theory is developed for one- and two-atom interactions when the atom has a Rydberg electron attached to a hyperfine-split core state. This situation is relevant for some of the rare-earth and alkaline-earth atoms that have been proposed for experiments on Rydberg-Rydberg interactions. For the rare-earth atoms, the core electrons can have a very substantial total angular momentum J and a nonzero nuclear spin I . In the alkaline-earth atoms there is a single (s ) core electron whose spin can couple to a nonzero nuclear spin for odd isotopes. The resulting hyperfine splitting of the core state can lead to substantial mixing between the Rydberg series attached to different thresholds. Compared to the unperturbed Rydberg series of the alkali-metal atoms, the series perturbations and near degeneracies from the different parity states could lead to qualitatively different behavior for single-atom Rydberg properties (polarizability, Zeeman mixing and splitting, etc.) as well as Rydberg-Rydberg interactions (C5 and C6 matrices).

Revivals of Rydberg wave packets

International Nuclear Information System (INIS)

Bluhm, R.; Kostelecky, V.A.; Tudose, B.

1998-01-01

We examine the revival structure of Rydberg wave packets. These wave packets exhibit initial classical periodic motion followed by a sequence of collapse, fractional (or full) revivals, and fractional (or full) superrevivals. The effects of quantum defects on wave packets in alkali-metal atoms and a squeezed-state description of the initial wave packets are also considered. We then examine the revival structure of Rydberg wave packets in the presence of an external electric field - that is, the revival structure of Stark wave packets. These wave packets have energies that depend on two quantum numbers and exhibit new types of interference behavior

Resonant inelastic x-ray scattering and photoemission measurement of O2: Direct evidence for dependence of Rydberg-valence mixing on vibrational states in O 1s → Rydberg states

Science.gov (United States)

Gejo, T.; Oura, M.; Tokushima, T.; Horikawa, Y.; Arai, H.; Shin, S.; Kimberg, V.; Kosugi, N.

2017-07-01

High-resolution resonant inelastic x-ray scattering (RIXS) and low-energy photoemission spectra of oxygen molecules have been measured for investigating the electronic structure of Rydberg states in the O 1s → σ* energy region. The electronic characteristics of each Rydberg state have been successfully observed, and new assignments are made for several states. The RIXS spectra clearly show that vibrational excitation is very sensitive to the electronic characteristics because of Rydberg-valence mixing and vibronic coupling in O2. This observation constitutes direct experimental evidence that the Rydberg-valence mixing characteristic depends on the vibrational excitation near the avoided crossing of potential surfaces. We also measured the photoemission spectra of metastable oxygen atoms (O*) from O2 excited to 1s → Rydberg states. The broadening of the 4p Rydberg states of O* has been found with isotropic behavior, implying that excited oxygen molecules undergo dissociation with a lifetime of the order of 10 fs in 1s → Rydberg states.

Scaling laws of Rydberg excitons

Science.gov (United States)

Heckötter, J.; Freitag, M.; Fröhlich, D.; Aßmann, M.; Bayer, M.; Semina, M. A.; Glazov, M. M.

2017-09-01

Rydberg atoms have attracted considerable interest due to their huge interaction among each other and with external fields. They demonstrate characteristic scaling laws in dependence on the principal quantum number n for features such as the magnetic field for level crossing or the electric field of dissociation. Recently, the observation of excitons in highly excited states has allowed studying Rydberg physics in cuprous oxide crystals. Fundamentally different insights may be expected for Rydberg excitons, as the crystal environment and associated symmetry reduction compared to vacuum give not only optical access to many more states within an exciton multiplet but also extend the Hamiltonian for describing the exciton beyond the hydrogen model. Here we study experimentally and theoretically the scaling of several parameters of Rydberg excitons with n , for some of which we indeed find laws different from those of atoms. For others we find identical scaling laws with n , even though their origin may be distinctly different from the atomic case. At zero field the energy splitting of a particular multiplet n scales as n-3 due to crystal-specific terms in the Hamiltonian, e.g., from the valence band structure. From absorption spectra in magnetic field we find for the first crossing of levels with adjacent principal quantum numbers a Br∝n-4 dependence of the resonance field strength, Br, due to the dominant paramagnetic term unlike for atoms for which the diamagnetic contribution is decisive, resulting in a Br∝n-6 dependence. By contrast, the resonance electric field strength shows a scaling as Er∝n-5 as for Rydberg atoms. Also similar to atoms with the exception of hydrogen we observe anticrossings between states belonging to multiplets with different principal quantum numbers at these resonances. The energy splittings at the avoided crossings scale roughly as n-4, again due to crystal specific features in the exciton Hamiltonian. The data also allow us to

Rydberg atoms ionization by microwave field and electromagnetic pulses

International Nuclear Information System (INIS)

Kaulakys, B.; Vilutis, G.

1995-01-01

A simple theory of the Rydberg atoms ionization by electromagnetic pulses and microwave field is presented. The analysis is based on the scale transformation which reduces the number of parameters and reveals the functional dependencies of the processes. It is shown that the observed ionization of Rydberg atoms by subpicosecond electromagnetic pulses scale classically. The threshold electric field required to ionise a Rydberg state may be simply evaluated in the photonic basis approach for the quantum dynamics or from the multiphoton ionization theory

Strontium-rubidium infusion pump with in-line dosimetry

International Nuclear Information System (INIS)

Barker, S.L.; Loberg, M.D.

1986-01-01

A strontium-rubidium infusion system is described which consists of: (a) means for generating rubidium 82 in a solution which can be infused into a patient; (b) means for infusing the solution into a patient; (c) means for measuring the radioactivity present in the solution as it is infused into the patient; and (d) means for controlling the means for infusing in response to the amount of radioactivity which has been infused into the patient

Contaminant-State Broadening Mechanism in a Driven Dissipative Rydberg System

Science.gov (United States)

Porto, J. V.

2017-04-01

The strong interactions in Rydberg atoms make them an ideal system for the study of correlated many-body physics, both in the presence and absence of dissipation. Using such highly excited atomic states requires addressing challenges posed by the dense spectrum of Rydberg levels, the detrimental effects of spontaneous emission, and strong interactions. A full understanding of the scope and limitations of many Rydberg-based proposals requires simultaneously including these effects, which typically cannot be described by a mean-field treatment due to correlations in the quantum coherent and dissipative processes. We study a driven, dissipative system of Rydberg atoms in a 3D optical lattice, and observe substantial deviation from single-particle excitation rates, both on and off resonance. The observed broadened spectra cannot be explained by van der Waals interactions or a mean-field treatment of the system. Based on the magnitude of the broadening and the scaling with density and two-photon Rabi frequency, we attribute these effects to unavoidable blackbody-induced transitions to nearby Rydberg states of opposite parity, which have large, resonant dipole-dipole interactions with the state of interest. Even at low densities of Rydberg atoms, uncontrolled production of atoms in other states significantly modifies the energy levels of the remaining atoms. These off-diagonal exchange interactions result in complex many-body states of the system and have implications for off-resonant Rydberg dressing proposals. This work was partially supported by the ARL-CDQI program.

Theoretical Analysis of Rydberg and Autoionizing State Spectra of Antimony

Institute of Scientific and Technical Information of China (English)

Shuang-Fei Lv; Ruohong Li; Feng-Dong Jia; Xiao-Kang Li; Jens Lassen; Zhi-Ping Zhong

2017-01-01

We calculate the Rydberg and autoionization Rydberg spectra of antimony (Sb) from first principles by relativistic multichannel theory within the framework of multichannel quantum defect theory.Our calculation can be used to classify and assign the atomic states described in recently reported three Rydberg series and four autoionizing states.The perturbation effects on line intensity,variation and line profile are discussed.Assignments of the perturber states and autoionizing states are presented.

Sympathetic cooling of nanospheres with cold atoms

Science.gov (United States)

Montoya, Cris; Witherspoon, Apryl; Ranjit, Gambhir; Casey, Kirsten; Kitching, John; Geraci, Andrew

2016-05-01

Ground state cooling of mesoscopic mechanical structures could enable new hybrid quantum systems where mechanical oscillators act as transducers. Such systems could provide coupling between photons, spins and charges via phonons. It has recently been shown theoretically that optically trapped dielectric nanospheres could reach the ground state via sympathetic cooling with trapped cold atoms. This technique can be beneficial in cases where cryogenic operation of the oscillator is not practical. We describe experimental advances towards coupling an optically levitated dielectric nanosphere to a gas of cold Rubidium atoms. The sphere and the cold atoms are in separate vacuum chambers and are coupled using a one-dimensional optical lattice. This work is partially supported by NSF, Grant Nos. PHY-1205994,PHY-1506431.

Simulation of coherent interactions between Rydberg atoms

International Nuclear Information System (INIS)

Robicheaux, F.; Hernandez, J.V.; Topcu, T.; Noordam, L.D.

2004-01-01

The results of a theoretical investigation of the coherent interaction between many Rydberg atoms are reported. The atoms are assumed to move very little during the time range we investigate. We describe the basic interaction between atoms and show that (contrary to previous theoretical studies) the interaction between the atoms can be coherent. The band structure for a perfect lattice of atoms and the density of states for an amorphous distribution of atoms are presented. We also give results for when the atoms are roughly positioned in a lattice. Finally, we performed detailed calculations to understand when the Rydberg interactions are too strong for an essential states type of approximation. The relevance of our results to previous measurements in a Rydberg gas and to possible future experiments is discussed

The effects of potassium and rubidium hydroxide on the alkali-silica reaction

International Nuclear Information System (INIS)

Shomglin, K.; Turanli, L.; Wenk, H.-R.; Monteiro, P.J.M.; Sposito, G.

2003-01-01

Expansion of mortar specimens prepared with an aggregate of mylonite from the Santa Rosa mylonite zone in southern California was studied to investigate the effect of different alkali ions on the alkali-silica reaction in concrete. The expansion tests indicate that mortar has a greater expansion when subjected to a sodium hydroxide bath than in a sodium-potassium-rubidium hydroxide bath. Electron probe microanalysis (EPMA) of mortar bars at early ages show that rubidium ions, used as tracer, were present throughout the sample by the third day of exposure. The analysis also shows a high concentration of rubidium in silica gel from mortar bars exposed to bath solutions containing rubidium. The results suggest that expansion of mortar bars using ASTM C 1260 does not depend on the diffusion of alkali ions. The results indicate that the expansion of alkali-silica gel depends on the type of alkali ions present. Alkali-silica gel containing rubidium shows a lower concentration of calcium, suggesting competition for the same sites

Synthesis of condensed double rubidium manganese phosphates in melts of polyphosphoric acids

International Nuclear Information System (INIS)

Guzeeva, L.S.; Tananaev, I.V.

1988-01-01

The aim of this work was to study the character of the reaction of MnO 2 and Rb 2 O with melts of polyphosphoric acids, and to establish the composition and the conditions of formation of the condensed double rubidium manganese phosphates. In the reaction of manganese and rubidium oxides with melts of polyphosphoric acids at 140-350 degree C, three types of trivalent manganese and rubidium condensed double phosphates are formed - diphosphates RbMn(H 2 P 2 O 7 ) and Rb 2 MnH 3 (P 2 O 7 ) 2 , triphosphate RbMnHP 3 O 10 and diphosphate RbMnP 2 O 7 - in addition to a double cyclotriphosphate of divalent manganese with rubidium RbMnP 3 O 9 . The thermal transformations of the compound isolated were studied. It was shown that rubidium manganese cyclotriphosphate can be obtained by the thermal decomposition of the diphosphate RbMn(H 2 P 2 O 7 ) 2

Self-interaction corrected density functional calculations of molecular Rydberg states

International Nuclear Information System (INIS)

Gudmundsdóttir, Hildur; Zhang, Yao; Weber, Peter M.; Jónsson, Hannes

2013-01-01

A method is presented for calculating the wave function and energy of Rydberg excited states of molecules. A good estimate of the Rydberg state orbital is obtained using ground state density functional theory including Perdew-Zunger self-interaction correction and an optimized effective potential. The total energy of the excited molecule is obtained using the Delta Self-Consistent Field method where an electron is removed from the highest occupied orbital and placed in the Rydberg orbital. Results are presented for the first few Rydberg states of NH 3 , H 2 O, H 2 CO, C 2 H 4 , and N(CH 3 ) 3 . The mean absolute error in the energy of the 33 molecular Rydberg states presented here is 0.18 eV. The orbitals are represented on a real space grid, avoiding the dependence on diffuse atomic basis sets. As in standard density functional theory calculations, the computational effort scales as NM 2 where N is the number of orbitals and M is the number of grid points included in the calculation. Due to the slow scaling of the computational effort with system size and the high level of parallelism in the real space grid approach, the method presented here makes it possible to estimate Rydberg electron binding energy in large molecules

Model potential for electron scattering from rubidium

Energy Technology Data Exchange (ETDEWEB)

Gien, T.E. (Memorial Univ. of Newfoundland, St. John' s, NF (Canada). Dept. of Physics)

1992-11-28

An analytic model potential for the e[sup -]-Rb[sup +] system is generated from experimental data, using an iteration method. The potential obtained can reproduce rather accurately the energy levels of rubidium. We employed it in the calculation of elastic differential cross sections for electron (and positron) scatterings from rubidium in the conventional Glauber approximation. The differential cross sections calculated in the model potential approach are compared to those in the frozen-core approach, employing either the Clementi-Roetti or the Szasz-McGinn wavefunctions. The core correlation and polarization effects are found to significantly affect the cross section results. (author).

Model potential for electron scattering from rubidium

International Nuclear Information System (INIS)

Gien, T.E.

1992-01-01

An analytic model potential for the e - -Rb + system is generated from experimental data, using an iteration method. The potential obtained can reproduce rather accurately the energy levels of rubidium. We employed it in the calculation of elastic differential cross sections for electron (and positron) scatterings from rubidium in the conventional Glauber approximation. The differential cross sections calculated in the model potential approach are compared to those in the frozen-core approach, employing either the Clementi-Roetti or the Szasz-McGinn wavefunctions. The core correlation and polarization effects are found to significantly affect the cross section results. (author)

Stimulated adiabatic passage in a dissipative ensemble of atoms with strong Rydberg-state interactions

DEFF Research Database (Denmark)

Petrosyan, David; Molmer, Klaus

2013-01-01

We study two-photon excitation of Rydberg states of atoms under stimulated adiabatic passage with delayed laser pulses. We find that the combination of strong interaction between the atoms in Rydberg state and the spontaneous decay of the intermediate exited atomic state leads to the Rydberg exci...... for deterministic creation and, possibly, extraction of Rydberg atoms or ions one at a time. The sympathetic monitoring via decay of ancilla particles may find wider applications for state preparation and probing of interactions in dissipative many-body systems.......We study two-photon excitation of Rydberg states of atoms under stimulated adiabatic passage with delayed laser pulses. We find that the combination of strong interaction between the atoms in Rydberg state and the spontaneous decay of the intermediate exited atomic state leads to the Rydberg...

Metastability and Rydberg states of triatomic hydrogen

International Nuclear Information System (INIS)

Helm, H.

1991-01-01

The np,nd and nf Rydberg series of H 3 have been studied by one- or two-photon excitation from the lowest metastable state of H 3 :B2p 2 A 2 ''. The lifetime of the metastable state has been measured and the influence of an external electric field on the Rydberg states has been studied under both aspects of dynamics (field-ionization and field-induced predissociation) and structure (Strak effect)

Robustness of high-fidelity Rydberg gates with single-site addressability

Science.gov (United States)

Goerz, Michael H.; Halperin, Eli J.; Aytac, Jon M.; Koch, Christiane P.; Whaley, K. Birgitta

2014-09-01

Controlled-phase (cphase) gates can be realized with trapped neutral atoms by making use of the Rydberg blockade. Achieving the ultrahigh fidelities required for quantum computation with such Rydberg gates, however, is compromised by experimental inaccuracies in pulse amplitudes and timings, as well as by stray fields that cause fluctuations of the Rydberg levels. We report here a comparative study of analytic and numerical pulse sequences for the Rydberg cphase gate that specifically examines the robustness of the gate fidelity with respect to such experimental perturbations. Analytical pulse sequences of both simultaneous and stimulated Raman adiabatic passage (STIRAP) are found to be at best moderately robust under these perturbations. In contrast, optimal control theory is seen to allow generation of numerical pulses that are inherently robust within a predefined tolerance window. The resulting numerical pulse shapes display simple modulation patterns and can be rationalized in terms of an interference between distinct two-photon Rydberg excitation pathways. Pulses of such low complexity should be experimentally feasible, allowing gate fidelities of order 99.90-99.99% to be achievable under realistic experimental conditions.

Transient localization in the kicked Rydberg atom

OpenAIRE

Persson, E.; Fürthauer, S.; Wimberger, S.; Burgdörfer, J.

2006-01-01

We investigate the long-time limit of quantum localization of the kicked Rydberg atom. The kicked Rydberg atom is shown to possess in addition to the quantum localization time $\\tau_L$ a second cross-over time $t_D$ where quantum dynamics diverges from classical dynamics towards increased instability. The quantum localization is shown to vanish as either the strength of the kicks at fixed principal quantum number or the quantum number at fixed kick strength increases. The survival probability...

Selective Bioaccumulation of Rubidium by Microalgae from Industrial Wastewater Containing Rubidium and Lithium.

Czech Academy of Sciences Publication Activity Database

Kaštánek, P.; Kronusová, O.; Kaštánek, František; Brányiková, Irena; Prochazková, G.; Jandová, J.; Brányik, T.; Bišová, Kateřina

2018-01-01

Roč. 30, č. 1 (2018), s. 461-467 ISSN 0921-8971 R&D Projects: GA TA ČR TE01020080 Institutional support: RVO:67985858 ; RVO:61388971 Keywords : rubidium * lithium * microalgae Subject RIV: CI - Industrial Chemistry, Chemical Engineering; EE - Microbiology, Virology (MBU-M) OBOR OECD: Chemical process engineering; Microbiology (MBU-M) Impact factor: 2.616, year: 2016

High resolution studies of barium Rydberg states

International Nuclear Information System (INIS)

Eliel, E.R.

1982-01-01

The subtle structure of Rydberg states of barium with orbital angular momentum 0, 1, 2 and 3 is investigated. Some aspects of atomic theory for a configuration with two valence electrons are reviewed. The Multi Channel Quantum Defect Theory (MQDT) is concisely introduced as a convenient way to describe interactions between Rydberg series. Three high-resolution UV studies are presented. The first two, presenting results on a transition in indium and europium serve as an illustration of the frequency doubling technique. The third study is of hyperfine structure and isotope shifts in low-lying p states in Sr and Ba. An extensive study of the 6snp and 6snf Rydberg states of barium is presented with particular emphasis on the 6snf states. It is shown that the level structure cannot be fully explained with the model introduced earlier. Rather an effective two-body spin-orbit interaction has to be introduced to account for the observed splittings, illustrating that high resolution studies on Rydberg states offer an unique opportunity to determine the importance of such effects. Finally, the 6sns and 6snd series are considered. The hyperfine induced isotope shift in the simple excitation spectra to 6sns 1 S 0 is discussed and attention is paid to series perturbers. It is shown that level mixing parameters can easily be extracted from the experimental data. (Auth.)

Shear viscosity of liquid argon and liquid rubidium

International Nuclear Information System (INIS)

Chiakwelu, O.

1978-01-01

A direct evaluation of the shear viscosity coefficient for models of liquid rubidium and liquid argon is presented by neglecting the cross-terms in the autocorrelation function of the transverse component of the momentum stress tensor. The time dependence of the shear viscosity for liquid argon is found to display a long decaying tail in qualitative agreement with a computer calculation of Levesque et al. However, the numerical values of the shear viscosity coefficients are smaller than the experimentally determined values of about 45% for liquid rubidium and 35% for liquid argon

Coherent Microwave-to-Optical Conversion via Six-Wave Mixing in Rydberg Atoms

Science.gov (United States)

Han, Jingshan; Vogt, Thibault; Gross, Christian; Jaksch, Dieter; Kiffner, Martin; Li, Wenhui

2018-03-01

We present an experimental demonstration of converting a microwave field to an optical field via frequency mixing in a cloud of cold 87Rb atoms, where the microwave field strongly couples to an electric dipole transition between Rydberg states. We show that the conversion allows the phase information of the microwave field to be coherently transferred to the optical field. With the current energy level scheme and experimental geometry, we achieve a photon-conversion efficiency of ˜0.3 % at low microwave intensities and a broad conversion bandwidth of more than 4 MHz. Theoretical simulations agree well with the experimental data, and they indicate that near-unit efficiency is possible in future experiments.

Many-body quantum simulation with Rydberg atoms and ions

International Nuclear Information System (INIS)

Mueller, M.

2010-01-01

This thesis presents my work that is located at the interface between the fields of atomic physics, quantum optics and quantum information. The work was performed at the Institute of Theoretical Physics of the University of Innsbruck and the Institute for Quantum Optics and Quantum Information of the Austrian Academy of Sciences under the supervision of Prof. Peter Zoller. The main topic of this thesis is the investigation of new schemes for quantum simulation of interacting many-body systems. The thesis is divided into three parts, which cover my work on i) chains of trapped Rydberg ions ii) quantum information processing and simulation with Rydberg atoms and iii) quantum simulation with ground state ions. The first part of this thesis is concerned with the study of Rydberg ions trapped in a linear Paul trap. The properties of ionic Rydberg states in the presence of the static and time-dependent electric trapping fields are investigated. First it is analyzed under which conditions laser-excited Rydberg ions can be trapped in a stable configuration. Furthermore, it is shown that strong dipole-dipole interactions among the ions can be achieved by microwave dressing fields. These interactions can give rise to dynamics of Rydberg excitations through the ion crystal, which take place on a nanosecond timescale and can be described by effective spin-models. In addition, it is discussed how to achieve fast two-qubit entangling gates between pairs of Rydberg ions. In the second part of this thesis, novel possibilities of using neutral Rydberg atoms for quantum-information processing and quantum simulation are investigated. A new scheme for a multi-atom quantum gate is proposed and theoretically analyzed. This parallelized gate allows one to entangle a mesoscopic ensemble of atoms with a single control atom in a single step, with high fidelity and on a microsecond time scale. The operation relies on strong and long-ranged interactions between Rydberg atoms triggering a

Observations on the Reliability of Rubidium Frequency Standards on Block 2/2A GPS Satellites

Science.gov (United States)

Dieter, Gary L.

1996-01-01

Currently, the block 2/2A Global Positioning System (GPS) satellites are equipped with two rubidium frequency standards. These frequency standards were originally intended to serve as the back-ups to two cesium frequency standards. As the constellation ages, the master Control Station is forced to initialize and increasing number or rubidium frequency standards. Unfortunately the operational use of these frequency standards has not lived up to initial expectations. Although the performance of these rubidium frequency standards has met and even exceeded GPS requirements, their reliability has not. The number of unscheduled outage times and the short operational lifetimes of the rubidium frequency standards compare poorly to the track record of the cesium frequency standards. Only a small number of rubidium frequency standards have actually been made operational. Of these, a large percentage have exhibited poor reliability. If this trend continues, it is unlikely that the rubidium frequency standards will help contribute to the navigation payload meeting program specification.

Erratum to: Selective Bioaccumulation of Rubidium by Microalgae from Industrial Wastewater Containing Rubidium and Lithium.

Czech Academy of Sciences Publication Activity Database

Kaštánek, P.; Kronusová, O.; Kaštánek, František; Brányiková, Irena; Prochazková, G.; Jandová, J.; Brányik, T.; Bišová, Kateřina

2018-01-01

Roč. 30, č. 1 (2018), s. 469 ISSN 0921-8971 Institutional support: RVO:67985858 ; RVO:61388971 Keywords : rubidium * lithium * microalgae Subject RIV: CI - Industrial Chemistry, Chemical Engineering; EE - Microbiology, Virology (MBU-M) OBOR OECD: Chemical process engineering; Microbiology (MBU-M) Impact factor: 2.616, year: 2016

Nonadiabatic holonomic quantum computation using Rydberg blockade

Science.gov (United States)

Kang, Yi-Hao; Chen, Ye-Hong; Shi, Zhi-Cheng; Huang, Bi-Hua; Song, Jie; Xia, Yan

2018-04-01

In this paper, we propose a scheme for realizing nonadiabatic holonomic computation assisted by two atoms and the shortcuts to adiabaticity (STA). The blockade effect induced by strong Rydberg-mediated interaction between two Rydberg atoms provides us the possibility to simplify the dynamics of the system, and the STA helps us design pulses for implementing the holonomic computation with high fidelity. Numerical simulations show the scheme is noise immune and decoherence resistant. Therefore, the current scheme may provide some useful perspectives for realizing nonadiabatic holonomic computation.

Strontium-82/rubidium-82 generator

International Nuclear Information System (INIS)

Gennaro, G.P.; Haney, P.S.

1986-01-01

Hydroxylapatite, a compound having the formula: M 10 (PO 4 ) 6 (OH) 2 wherein M is calcium, strontium, barium, lead, iron, sodium, potassium, zinc, cadmium, magnesium, aluminium or a rare earth metal, is provided as a support medium for strontium-82 in a strontium-82/rubidium-82 parent-daughter radionuclide generator

Spontaneuos and Parametric Processes in Warm Rubidium Vapours

Directory of Open Access Journals (Sweden)

Dąbrowski M.

2014-12-01

Full Text Available Warm rubidium vapours are known to be a versatile medium for a variety of experiments in atomic physics and quantum optics. Here we present experimental results on producing the frequency converted light for quantum applications based on spontaneous and stimulated processes in rubidium vapours. In particular, we study the efficiency of spontaneously initiated stimulated Raman scattering in the Λ-level configuration and conditions of generating the coherent blue light assisted by multi-photon transitions in the diamond-level configuration. Our results will be helpful in search for new types of interfaces between light and atomic quantum memories.

Ionization of Rydberg atoms by the kicks of half-cycle pulses

Indian Academy of Sciences (India)

Rydberg atom; half-cycle pulses; ionization; quantum mechanical model. ... packet which represents a non-stationary quantum state formed by coherent ...... Wetzels, Impulsive interactions of half cycle pulse radiation with Rydberg atoms, Ph.D.

Bichromatic electromagnetically induced transparency in cold rubidium atoms

International Nuclear Information System (INIS)

Wang, J.; Jiang, K.J.; Zhan, M.S.; Zhu Yifu

2003-01-01

In a three-level atomic system coupled by two equal-amplitude laser fields with a frequency separation 2δ, a weak probe field exhibits a multiple-peaked absorption spectrum with a constant peak separation δ. The corresponding probe dispersion exhibits steep normal dispersion near the minimum absorption between the multiple absorption peaks, which leads to simultaneous slow group velocities for probe photons at multiple frequencies separated by δ. We report an experimental study in such a bichromatically coupled three-level Λ system in cold 87 Rb atoms. The multiple-peaked probe absorption spectra under various experimental conditions have been observed and compared with the theoretical calculations

Non-selective photoionization of Rubidium

International Nuclear Information System (INIS)

1987-01-01

Effusive atomic beam of Rubidium have been generated through an effusive source. An oriel uv-light source was focused to irradiate and interact with atomic beam of Rb. The energy of the uv-lamp was enough to raise the Rb atom by 4.17 eV to the ionization continuum level of Rb

Electromagnetically induced transparency in thermal Rydberg atoms: superatom model with finite Doppler broadening

Science.gov (United States)

Bai, Si-Yin; Bao, Qian-Qian; Tian, Xue-Dong; Liu, Yi-Mou; Wu, Jin-Hui

2018-04-01

We study the steady optical responses of a cold atomic ensemble driven into the three-level ladder configuration involving a Rydberg state at finite temperatures. By improving the superatom model with thermal movement included, we calculate relevant atomic coherence effects and find that the residual Doppler broadening at the mK-K temperatures will weaken the nonclassical properties of transmitted probe photons. Furthermore, propagation directions of the probe and coupling fields have a great influence on various properties related to electromagnetically induced transparency. That is, the residual Doppler effect is more destructive to relevant atomic coherence effects in the co-propagation case but can be partially eliminated in the counter-propagation case.

Evidence of Antiblockade in an Ultracold Rydberg Gas

Science.gov (United States)

Amthor, Thomas; Giese, Christian; Hofmann, Christoph S.; Weidemüller, Matthias

2010-01-01

We present the experimental observation of the antiblockade in an ultracold Rydberg gas recently proposed by Ates et al. [Phys. Rev. Lett. 98, 023002 (2007)PRLTAO0031-900710.1103/PhysRevLett.98.023002]. Our approach allows the control of the pair distribution in the gas and is based on a strong coupling of one transition in an atomic three-level system, while introducing specific detunings of the other transition. When the coupling energy matches the interaction energy of the Rydberg long-range interactions, the otherwise blocked excitation of close pairs becomes possible. A time-resolved spectroscopic measurement of the Penning ionization signal is used to identify slight variations in the Rydberg pair distribution of a random arrangement of atoms. A model based on a pair interaction Hamiltonian is presented which well reproduces our experimental observations and allows one to deduce the distribution of nearest-neighbor distances.

Precision flow-controlled rubidium-82 generator for bolus and constant infusion studies

International Nuclear Information System (INIS)

Yano, Y.

1981-01-01

A unique flow rate controller and large reservoir pumping system have been developed for infusing rubidium-82 intravenously at bolus, constant, or variable infusion rates. Using rubidium-82 and the positron ring detector tomograph, extraction or flow information can be obtained in studies of the heart, head, or kidneys

Molecular Rydberg transitions in carbon monoxide

International Nuclear Information System (INIS)

Fock, J.H.; Guertler, P.; Koch, E.E.

1979-10-01

The linear correlation between the term value and ionization energy for molecular Rydberg transitions is tested for the sequence of isoelectronic molecules BF, CO and N 2 based on a new measurement of the absorption spectrum of CO and data for BF and N 2 . For the npsigma series and npπ series converging on the first ionization potential, we find an excellent linear behavior (within 10 meV) corroborating (I) the correlation and (II) the individual assignments. For Rydberg series leading to the A 2 DELTA and B 2 EPSILON + states, where no data for BF are available, a comparison of term values for CO and N 2 is presented. (orig.)

Microscopic Characterization of Scalable Coherent Rydberg Superatoms

Directory of Open Access Journals (Sweden)

Johannes Zeiher

2015-08-01

Full Text Available Strong interactions can amplify quantum effects such that they become important on macroscopic scales. Controlling these coherently on a single-particle level is essential for the tailored preparation of strongly correlated quantum systems and opens up new prospects for quantum technologies. Rydberg atoms offer such strong interactions, which lead to extreme nonlinearities in laser-coupled atomic ensembles. As a result, multiple excitation of a micrometer-sized cloud can be blocked while the light-matter coupling becomes collectively enhanced. The resulting two-level system, often called a “superatom,” is a valuable resource for quantum information, providing a collective qubit. Here, we report on the preparation of 2 orders of magnitude scalable superatoms utilizing the large interaction strength provided by Rydberg atoms combined with precise control of an ensemble of ultracold atoms in an optical lattice. The latter is achieved with sub-shot-noise precision by local manipulation of a two-dimensional Mott insulator. We microscopically confirm the superatom picture by in situ detection of the Rydberg excitations and observe the characteristic square-root scaling of the optical coupling with the number of atoms. Enabled by the full control over the atomic sample, including the motional degrees of freedom, we infer the overlap of the produced many-body state with a W state from the observed Rabi oscillations and deduce the presence of entanglement. Finally, we investigate the breakdown of the superatom picture when two Rydberg excitations are present in the system, which leads to dephasing and a loss of coherence.

The Kinetics of Ouabain Inhibition and the Partition of Rubidium Influx in Human Red Blood Cells

Science.gov (United States)

Beauge, L. A.; Adragna, Norma

1971-01-01

In the development of ouabain inhibition of rubidium influx in human red blood cells a time lag can be detected which is a function of at least three variables: the concentrations of external sodium, rubidium, and ouabain. The inhibition is antagonized by rubidium and favored by sodium. Similar considerations could be applied to the binding of ouabain to membrane sites. The total influx of rubidium as a function of external rubidium concentration can be separated into two components: (a) a linear uptake not affected by external sodium or ouabain and not requiring an energy supply, and (b) a saturable component. The latter component, on the basis of the different effects of the aforementioned factors, can be divided into three fractions. The first is ouabain-sensitive, inhibited by external sodium at low rubidium, and requires an energy supply; this represents about 70–80% of the total uptake and is related to the active sodium extrusion mechanism. The second is ouabain-insensitive, activated by external sodium over the entire range of rubidium concentrations studied, and dependent on internal ATP; this represents about 15% of the total influx; it could be coupled to an active sodium extrusion or belong to a rubidium-potassium exchange. The third, which can be called residual influx, is ouabain-insensitive, unaffected by external sodium, and independent of internal ATP; this represents about 10–20% of the total influx. PMID:5553102

Transient localization in the kicked Rydberg atom

International Nuclear Information System (INIS)

Persson, Emil; Fuerthauer, S.; Burgdoerfer, J.; Wimberger, S.

2006-01-01

We investigate the long-time limit of quantum localization of the kicked Rydberg atom. The kicked Rydberg atom is shown to possess in addition to the quantum localization time τ L a second crossover time t D where quantum dynamics diverges from classical dynamics towards increased instability. The quantum localization is shown to vanish as either the strength of the kicks at fixed principal quantum number or the quantum number at fixed kick strength increases. The survival probability as a function of frequency in the transient localization regime τ L D is characterized by highly irregular, fractal-like fluctuations

Interactions of circular Rydberg atoms with charged particles

International Nuclear Information System (INIS)

Wang, J.

1994-01-01

Recent progress in experimental cross-field techniques has made it possible to produce oriented Rydberg atoms of any angular momentum l within a given n manifold. The largest angular momentum state l max = n - 1 of a given n manifold is of particular interest because of its semiclassical properties for n much-gt 1. The corresponding classical Kepler orbit is circular with highly localized phase space distribution. The circular Rydberg atoms afford the opportunity to study various interactions in the semiclassical regime. The authors report electron capture from circular Rydberg atoms by protons and positrons at speeds comparable to the electron orbital speed. They find orientation dependent, novel peak structures for both protons and positrons in the angular scattering of the particles. The structures may be understood in terms of quasi Thomas double scattering mechanism for capture. Other related aspects including final state population and orientation indulged scattering asymmetry will also be discussed

Observation of pendular butterfly Rydberg molecules

Science.gov (United States)

Niederprüm, Thomas; Thomas, Oliver; Eichert, Tanita; Lippe, Carsten; Pérez-Ríos, Jesús; Greene, Chris H.; Ott, Herwig

2016-01-01

Engineering molecules with a tunable bond length and defined quantum states lies at the heart of quantum chemistry. The unconventional binding mechanism of Rydberg molecules makes them a promising candidate to implement such tunable molecules. A very peculiar type of Rydberg molecules are the so-called butterfly molecules, which are bound by a shape resonance in the electron–perturber scattering. Here we report the observation of these exotic molecules and employ their exceptional properties to engineer their bond length, vibrational state, angular momentum and orientation in a small electric field. Combining the variable bond length with their giant dipole moment of several hundred Debye, we observe counter-intuitive molecules which locate the average electron position beyond the internuclear distance. PMID:27703143

Correlated Photon Emission from Multiatom Rydberg Dark States

DEFF Research Database (Denmark)

Pritchard, J.D.; Adams, C.S.; Mølmer, Klaus

2012-01-01

We consider three-level atoms driven by two resonant light fields in a ladder scheme where the upper level is a highly excited Rydberg state. We show that the dipole-dipole interactions between Rydberg excited atoms prevents the formation of single particle dark states and leads to strongly corre...... correlated photon pairs from atoms separated by distances large compared to the emission wavelength. For a pair of atoms, this enables realization of an efficient photon-pair source with on average one pair every 30 μs....

Semiclassical calculation of ionisation rate for Rydberg helium atoms in an electric field

International Nuclear Information System (INIS)

Wang De-Hua

2011-01-01

The ionisation of Rydberg helium atoms in an electric field above the classical ionisation threshold has been examined using the semiclassical method, with particular emphasis on discussing the influence of the core scattering on the escape dynamics of electrons. The results show that the Rydberg helium atoms ionise by emitting a train of electron pulses. Unlike the case of the ionisation of Rydberg hydrogen atom in parallel electric and magnetic fields, where the pulses of the electron are caused by the external magnetic field, the pulse trains for Rydberg helium atoms are created through core scattering. Each peak in the ionisation rate corresponds to the contribution of one core-scattered combination trajectory. This fact further illustrates that the ionic core scattering leads to the chaotic property of the Rydberg helium atom in external fields. Our studies provide a simple explanation for the escape dynamics in the ionisation of nonhydrogenic atoms in external fields. (atomic and molecular physics)

Velocity-selective dark states in rubidium

International Nuclear Information System (INIS)

Esslinger, T.

1995-06-01

There are two recent developments exerting a strong influence on atomic physics: cooling of atomic gases with laser light, and optics with matter waves. The report addresses both fields. A mechanism for the cooling of atoms is examined, with the wave character of the atom playing an important part in the process. A novel atomic beam experiment has been worked out and is reported which represents application of this cooling method to an alkali atom for the first time. The basic principle of the cooling process is that atoms are optically pumped into quantum states by means of interaction with a standing laser wave, the quantum states having a sharply defined momentum, decoupled from the light field. These states are called dark states, as their dipole moment does not couple to the field of a resonant laser wave. In a one-dimensional standing laser wave with spatially varying polarization, the dark state is delocalised. This state is called velocity-selective dark state (VSDS). So far, such VSDS have only been observed in helium atoms. We succeded for the first time in detecting the population of VSDS with an experiment using alkali atoms. Atoms of a cold rubidium beam are optically pumped into VSDS by way of interaction with a one-dimensional standing laser wave. (orig./MM) [de

Cavity electromagnetically induced transparency with Rydberg atoms

Science.gov (United States)

Bakar Ali, Abu; Ziauddin

2018-02-01

Cavity electromagnetically induced transparency (EIT) is revisited via the input probe field intensity. A strongly interacting Rydberg atomic medium ensemble is considered in a cavity, where atoms behave as superatoms (SAs) under the dipole blockade mechanism. Each atom in the strongly interacting Rydberg atomic medium (87 Rb) follows a three-level cascade atomic configuration. A strong control and weak probe field are employed in the cavity with the ensemble of Rydberg atoms. The features of the reflected and transmitted probe light are studied under the influence of the input probe field intensity. A transparency peak (cavity EIT) is revealed at a resonance condition for small values of input probe field intensity. The manipulation of the cavity EIT is reported by tuning the strength of the input probe field intensity. Further, the phase and group delay of the transmitted and reflected probe light are studied. It is found that group delay and phase in the reflected light are negative, while for the transmitted light they are positive. The magnitude control of group delay in the transmitted and reflected light is investigated via the input probe field intensity.

Rydberg energies using excited state density functional theory

International Nuclear Information System (INIS)

Cheng, C.-L.; Wu Qin; Van Voorhis, Troy

2008-01-01

We utilize excited state density functional theory (eDFT) to study Rydberg states in atoms. We show both analytically and numerically that semilocal functionals can give quite reasonable Rydberg energies from eDFT, even in cases where time dependent density functional theory (TDDFT) fails catastrophically. We trace these findings to the fact that in eDFT the Kohn-Sham potential for each state is computed using the appropriate excited state density. Unlike the ground state potential, which typically falls off exponentially, the sequence of excited state potentials has a component that falls off polynomially with distance, leading to a Rydberg-type series. We also address the rigorous basis of eDFT for these systems. Perdew and Levy have shown using the constrained search formalism that every stationary density corresponds, in principle, to an exact stationary state of the full many-body Hamiltonian. In the present context, this means that the excited state DFT solutions are rigorous as long as they deliver the minimum noninteracting kinetic energy for the given density. We use optimized effective potential techniques to show that, in some cases, the eDFT Rydberg solutions appear to deliver the minimum kinetic energy because the associated density is not pure state v-representable. We thus find that eDFT plays a complementary role to constrained DFT: The former works only if the excited state density is not the ground state of some potential while the latter applies only when the density is a ground state density.

Controlling stray electric fields on an atom chip for experiments on Rydberg atoms

Science.gov (United States)

Davtyan, D.; Machluf, S.; Soudijn, M. L.; Naber, J. B.; van Druten, N. J.; van Linden van den Heuvell, H. B.; Spreeuw, R. J. C.

2018-02-01

Experiments handling Rydberg atoms near surfaces must necessarily deal with the high sensitivity of Rydberg atoms to (stray) electric fields that typically emanate from adsorbates on the surface. We demonstrate a method to modify and reduce the stray electric field by changing the adsorbate distribution. We use one of the Rydberg excitation lasers to locally affect the adsorbed dipole distribution. By adjusting the averaged exposure time we change the strength (with the minimal value less than 0.2 V /cm at 78 μ m from the chip) and even the sign of the perpendicular field component. This technique is a useful tool for experiments handling Rydberg atoms near surfaces, including atom chips.

High-fidelity Rydberg quantum gate via a two-atom dark state

DEFF Research Database (Denmark)

Petrosyan, David; Motzoi, Felix; Saffman, Mark

2017-01-01

We propose a two-qubit gate for neutral atoms in which one of the logical state components adiabatically follows a two-atom dark state formed by the laser coupling to a Rydberg state and a strong, resonant dipole-dipole exchange interaction between two Rydberg excited atoms. Our gate exhibits...

Positron scattering by rubidium and caesium

International Nuclear Information System (INIS)

Kernoghan, A.A.; Walters, H.R.J.; McAlinden, M.T.

1996-01-01

We report results in the energy range 0.5 to 64 eV for positron scattering by ground state rubidium and caesium in Ps(1s,2s,2p,3s,3p,3d) + Rb(5s,5p,6s,6p,4d) and Ps(1s,2s,2p,3s,3p,3d) + Cs(6s,6p,7s,7p,5d) coupled-state approximations, respectively. The pattern of results is similar to analogous calculations made on potassium by McAlinden et al. Except at the lowest energies, positronium formation is found to be almost entirely into excited states, with there being a dramatic collapse of the Ps(1s) cross section in the case of caesium. Ps(n = 2), Ps(n = 3) and Ps(n≥ 4) cross sections are predicted to be of comparable size. Ps(n≥ 4) formation is estimated from the calculated Ps(n = 3) results using the n 3 scaling rule. Good agreement in shape and magnitude is obtained with the recent lower bound measurements of total positronium formation in rubidium by Surdutovich et al, although there are differences in detail. Good agreement is also achieved with the total cross section measurements of Parikh et al on rubidium after these have been corrected for discrimination against forward elastic scattering and renormalized upwards by 5%. These total cross section measurements display a pronounced peak near 6 eV which is well reproduced by the present theory but is at variance with the earlier Rb(5s,5p,6s,6p,4d) calculations of McEachran et al which neglect positronium formation. This peak, which also appears in the calculations on potassium and caesium, is primarily associated with the maximum in the total positronium formation cross section. At low energies elastic scattering is dominant, this dominance being directly taken over by the resonance excitation of the atom with increasing impact energy. The next most important cross section is positronium formation, followed by excitation of the lowest atomic d-state. The 5s → 6s and 5s → 6p transitions in rubidium and the 6s → 7s and 6s → 7p transitions in caesium are of relatively minor importance. (Author)

Two photon spectroscopy of rubidium atoms in a magneto-optic trap

International Nuclear Information System (INIS)

Fretel, E.

1997-01-01

Two photon transitions without doppler effect can be used as an atomic reference. The aim of this work is to study two photon transitions of rubidium atoms in a magneto-optical trap. The chosen transition is from the level 5 2 S 1/2 toward the level 5 2 D 5/2 . The magneto-optical trap is achieved by using 3 pairs of perpendicular laser beams and by setting a magnetic field gradient. About 10 18 atoms are trapped and cooled in a 1 mm 3 volume. In a first stage we have realized an optical double resonance experiment from the level 5 2 S 1/2 toward the level 5 2 D 5/2 by populating the intermediate level 5 2 P 3/2 . Then we have studied the two photon transition in this cluster of cold atoms. A particular setting of the experiment allows to reduce the effect of ray broadening and shifting due to the magnetic field of the trap

Wave-packet approach to Rydberg resonances in dissociative recombination

International Nuclear Information System (INIS)

Morisset, Sabine; Pichl, Lukas; Orel, Ann E.; Schneider, Ioan F.

2007-01-01

We report the time-dependent approach to resonant electron capture into Rydberg states in collisions with molecular cations at low impact energy, as an alternative to the method based on multichannel quantum defect theory (MQDT), and present the results for the HD + ion. The propagation of the initial wave function on 13 Rydberg states (besides one valence state) correctly describes the indirect dissociative recombination mechanism in the time domain. Notably, the nonlocal coupling operator between the ionization and dissociation channels is accounted for in the indirect process, extending previous work on the case of direct coupling. The present approach compares to the MQDT framework with remarkable precision: resonant structures in the cross section correctly emerge from the wave-packet propagation; the time-dependent result also forms a cross section envelope for the dense series of ultrafine MQDT resonances corresponding to the quasicontinuous part of the Rydberg state manifold

Many-body dynamics of holes in a driven, dissipative spin chain of Rydberg superatoms

Science.gov (United States)

Letscher, Fabian; Petrosyan, David; Fleischhauer, Michael

2017-11-01

Strong, long-range interactions between atoms in high-lying Rydberg states can suppress multiple Rydberg excitations within a micron-sized trapping volume and yield sizable Rydberg level shifts at larger distances. Ensembles of atoms in optical microtraps then form Rydberg superatoms with collectively enhanced transition rates to the singly excited state. These superatoms can represent mesoscopic, strongly interacting spins. We study a regular array of such effective spins driven by a laser field tuned to compensate the interaction-induced level shifts between neighboring superatoms. During the initial transient, a few excited superatoms seed a cascade of resonantly facilitated excitation of large clusters of superatoms. Due to spontaneous decay, the system then relaxes to the steady state having nearly universal Rydberg excitation density {ρ }{{R}}=2/3. This state is characterized by highly non-trivial equilibrium dynamics of quasi-particles—excitation holes in the lattice of Rydberg excited superatoms. We derive an effective many-body model that accounts for hole mobility as well as continuous creation and annihilation of holes upon collisions with each other. We find that holes exhibit a nearly incompressible liquid phase with highly sub-Poissonian number statistics and finite-range density-density correlations.

Dynamics of Rydberg atom lattices in the presence of noise and dissipation

International Nuclear Information System (INIS)

Abdussalam, Wildan

2017-01-01

The work presented in this dissertation concerns dynamics of Rydberg atom lattices in the presence of noise and dissipation. Rydberg atoms possess a number of exaggerated properties, such as a strong van der Waals interaction. The interplay of that interaction, coherent driving and decoherence leads to intriguing non-equilibrium phenomena. Here, we study the non-equilibrium physics of driven atom lattices in the presence of decoherence caused by either laser phase noise or strong decay. In the first case, we compare between global and local noise and explore their effect on the number of excitations and the full counting statistics. We find that both types of noise give rise to a characteristic distribution of the Rydberg excitation number. The main method employed is the Langevin equation but for the sake of efficiency in certain regimes, we use a Markovian master equation and Monte Carlo rate equations, respectively. In the second case, we consider dissipative systems with more general power-law interactions. We determine the phase diagram in the steady state and analyse its generation dynamics using Monte Carlo rate equations. In contrast to nearest-neighbour models, there is no transition to long-range-ordered phases for realistic interactions and resonant driving. Yet, for finite laser detunings, we show that Rydberg atom lattices can undergo a dissipative phase transition to a long-range-ordered antiferromagnetic phase. We identify the advantages of Monte Carlo rate equations over mean field predictions. Having studied the dynamics of Rydberg atom lattices, we study an application of the strong interactions in such systems for quantum information processing. We investigate the coherent exchange of a single photon between a superconducting microwave cavity and a lattice of strongly interacting Rydberg atoms in the presence of local electric field fluctuations plaguing the cavity surface. We show that despite the increased sensitivity of Rydberg states to

Dynamics of Rydberg atom lattices in the presence of noise and dissipation

Energy Technology Data Exchange (ETDEWEB)

Abdussalam, Wildan

2017-08-07

The work presented in this dissertation concerns dynamics of Rydberg atom lattices in the presence of noise and dissipation. Rydberg atoms possess a number of exaggerated properties, such as a strong van der Waals interaction. The interplay of that interaction, coherent driving and decoherence leads to intriguing non-equilibrium phenomena. Here, we study the non-equilibrium physics of driven atom lattices in the presence of decoherence caused by either laser phase noise or strong decay. In the first case, we compare between global and local noise and explore their effect on the number of excitations and the full counting statistics. We find that both types of noise give rise to a characteristic distribution of the Rydberg excitation number. The main method employed is the Langevin equation but for the sake of efficiency in certain regimes, we use a Markovian master equation and Monte Carlo rate equations, respectively. In the second case, we consider dissipative systems with more general power-law interactions. We determine the phase diagram in the steady state and analyse its generation dynamics using Monte Carlo rate equations. In contrast to nearest-neighbour models, there is no transition to long-range-ordered phases for realistic interactions and resonant driving. Yet, for finite laser detunings, we show that Rydberg atom lattices can undergo a dissipative phase transition to a long-range-ordered antiferromagnetic phase. We identify the advantages of Monte Carlo rate equations over mean field predictions. Having studied the dynamics of Rydberg atom lattices, we study an application of the strong interactions in such systems for quantum information processing. We investigate the coherent exchange of a single photon between a superconducting microwave cavity and a lattice of strongly interacting Rydberg atoms in the presence of local electric field fluctuations plaguing the cavity surface. We show that despite the increased sensitivity of Rydberg states to

Rydberg-state reionization of multiply charged ions escaping from solid surfaces

International Nuclear Information System (INIS)

Nedeljkovic, Lj.D.; Nedeljkovic, N.N.

2003-01-01

Reionization rates of Rydberg states (n>>1 and l=0, 1, and 2) of multiply charged ionic projectiles escaping solid surfaces are calculated. These rates are obtained in an analytic form as a function of the ion-surface distance R. A phenomenological model of the reionization process, based on two-state quantum dynamics, is adopted for the vicinity of the potential barrier top. The results of calculations show that ionization rates for different Rydberg states are strictly localized and relatively separated. Universality of the reionization rate as a function of the scaling parameter α, describing the turning point configurations, is demonstrated. The reionization is discussed within the framework of a nonresonant population-reionization process at intermediate ionic velocities (v∼1 a.u.). The influence of reionization on the population of ionic Rydberg states is expressed in terms of a renormalized neutralization rate. It is demonstrated that the reionization effect significantly changes the population curves for all Rydberg states. The population curves obtained correlate with beam-foil experimental data concerning the S VI, Cl VII, and Ar VIII ions

Autoionizing np Rydberg states of H2

International Nuclear Information System (INIS)

Xu, E.Y.; Helm, H.; Kachru, R.

1989-01-01

We report a study of the autoionizing np Rydberg states near the lowest ionization threshold of H 2 . Using resonant two-photon excitation, intermediate states in specific rotovibrational levels in the double well, E,F 1 Σ/sub g/ + states are prepared. Then, a second, tunable laser is used to photoionize via excitation of the np Rydberg states. Because of the stepwise laser excitation scheme employed in our experiment the photoionization occurs from states with vibrational wave functions very similar to those of the H 2 + core. As a consequence, the autoionizing states appear as nearly symmetric resonances, rather than the highly asymmetric Beutler-Fano profiles observed from the direct photoexcitation from the ground state of H 2 . Our experiments show that the J = 1 np states are broader than the J = 3 np states converging to the same limit, suggesting that the two states autoionize into the epsilon-cp and epsilon-cf continuum, respectively. We compare our observations with a theoretical analysis using a multichannel quantum defect theory. The J = 1 states reveal the profound effect caused by the perturbation of the autoionizing Rydberg series converging to the lowest vibrational and rotational state of H 2 + by low-n states converging to higher vibrational states of the H 2 -ion core

Trojan wavepackets in helium - by core-Rydberg interaction

International Nuclear Information System (INIS)

Kalinski, M.; Eberly, J.H.

1996-01-01

The authors exhibit the existence of core-induced shape invariant wave packets in helium analogous to the Trojan wave packets predicted for hydrogen. They show that the core dipole moment oscillating with the Rabi frequency in the presence of a laser field will cause both radical and angular confinement of an outer Rydberg electron moving around a nearly circular orbit if the parameters of the orbit are properly chosen. They find the relation between the Rabi frequency of the core electron oscillations, laser field strength and the parameters of the Rydberg orbit of the outer electron

Line shapes and time dynamics of the Förster resonances between two Rydberg atoms in a time-varying electric field

KAUST Repository

Yakshina, E. A.

2016-10-21

The observation of the Stark-tuned Förster resonances between Rydberg atoms excited by narrowband cw laser radiation requires usage of a Stark-switching technique in order to excite the atoms first in a fixed electric field and then to induce the interactions in a varied electric field, which is scanned across the Förster resonance. In our experiments with a few cold Rb Rydberg atoms, we have found that the transients at the edges of the electric pulses strongly affect the line shapes of the Förster resonances, since the population transfer at the resonances occurs on a time scale of ∼100 ns, which is comparable with the duration of the transients. For example, a short-term ringing at a certain frequency causes additional radio-frequency-assisted Förster resonances, while nonsharp edges lead to asymmetry. The intentional application of the radio-frequency field induces transitions between collective states, whose line shape depends on the interaction strengths and time. Spatial averaging over the atom positions in a single interaction volume yields a cusped line shape of the Förster resonance. We present a detailed experimental and theoretical analysis of the line shape and time dynamics of the Stark-tuned Förster resonances Rb(nP3/2)+Rb(nP3/2)→Rb(nS1/2)+Rb([n+1]S1/2) for two Rb Rydberg atoms interacting in a time-varying electric field.

Line shapes and time dynamics of the Förster resonances between two Rydberg atoms in a time-varying electric field

KAUST Repository

Yakshina, E. A.; Tretyakov, D. B.; Beterov, I. I.; Entin, V. M.; Andreeva, C.; Cinins, A.; Markovski, A.; Iftikhar, Z.; Ekers, Aigars; Ryabtsev, I. I.

2016-01-01

The observation of the Stark-tuned Förster resonances between Rydberg atoms excited by narrowband cw laser radiation requires usage of a Stark-switching technique in order to excite the atoms first in a fixed electric field and then to induce the interactions in a varied electric field, which is scanned across the Förster resonance. In our experiments with a few cold Rb Rydberg atoms, we have found that the transients at the edges of the electric pulses strongly affect the line shapes of the Förster resonances, since the population transfer at the resonances occurs on a time scale of ∼100 ns, which is comparable with the duration of the transients. For example, a short-term ringing at a certain frequency causes additional radio-frequency-assisted Förster resonances, while nonsharp edges lead to asymmetry. The intentional application of the radio-frequency field induces transitions between collective states, whose line shape depends on the interaction strengths and time. Spatial averaging over the atom positions in a single interaction volume yields a cusped line shape of the Förster resonance. We present a detailed experimental and theoretical analysis of the line shape and time dynamics of the Stark-tuned Förster resonances Rb(nP3/2)+Rb(nP3/2)→Rb(nS1/2)+Rb([n+1]S1/2) for two Rb Rydberg atoms interacting in a time-varying electric field.

Newton's Cradle and Entanglement Transport in a Flexible Rydberg Chain

International Nuclear Information System (INIS)

Wuester, S.; Ates, C.; Eisfeld, A.; Rost, J. M.

2010-01-01

In a regular, flexible chain of Rydberg atoms, a single electronic excitation localizes on two atoms that are in closer mutual proximity than all others. We show how the interplay between excitonic and atomic motion causes electronic excitation and diatomic proximity to propagate through the Rydberg chain as a combined pulse. In this manner entanglement is transferred adiabatically along the chain, reminiscent of momentum transfer in Newton's cradle.

Wavepacket dynamics of a Rydberg atom monitored by a pair of time-delayed laser pulses

Science.gov (United States)

Xin, PeiPei; Cheng, Hong; Zhang, ShanShan; Wang, HanMu; Liu, HongPing

2018-02-01

We have investigated the Rydberg state population of an argon atom by an intense laser pulse and its wavepacket dynamics monitored by another successive laser pulse in the tunneling regime. A wavepacket comprising a superposition of close high-lying Rydberg states is irradiated by a multicycle laser pulse, where the sub-wave components in the wavepacket have fixed relative phases. A time-delayed second laser pulse is employed to apply on the excited Rydberg atom. If the time is properly chosen, one of the sub-wave components will be guided towards the ionization area while the rest remains intact. By means of this pump-probe technique, we could control and monitor the Rydberg wavepacket dynamics and reveal some interesting phenomenon such as the survival rate of individual Rydberg states related to the classical orbital period of electron.

Excitation of higher lying energy states in a rubidium DPAL

Science.gov (United States)

Wallerstein, A. J.; Perram, Glen; Rice, Christopher A.

2018-02-01

The spontaneous emission in a cw rubidium diode dumped alkali laser (DPAL) system was analyzed. The fluorescence from higher lying states decreases with additional buffer gas. The intermediate states (7S, 6P, 5D) decay more slowly with buffer gas and scale super-linearly with alkali density. A detailed kinetic model has been constructed, where the dominant mechanisms are energy pooling and single photon ionization. It also includes pumping into the non-Lorentzian wings of absorption profiles, fine structure mixing, collisional de-excitation, and Penning ionization. Effects of ionization in a high powered CW rubidium DPAL were assessed.

Multibit C_kNOT quantum gates via Rydberg blockade

DEFF Research Database (Denmark)

Isenhower, L.; Saffman, Mark; Mølmer, Klaus

2011-01-01

Long range Rydberg blockade interactions have the potential for efficient implementation of quantum gates between multiple atoms. Here we present and analyze a protocol for implementation of a k-atom controlled NOT (CkNOT) neutral atom gate. This gate can be implemented using sequential or simult......Long range Rydberg blockade interactions have the potential for efficient implementation of quantum gates between multiple atoms. Here we present and analyze a protocol for implementation of a k-atom controlled NOT (CkNOT) neutral atom gate. This gate can be implemented using sequential...... or simultaneous addressing of the control atoms which requires only 2k + 3 or 5 Rydberg π pulses respectively. A detailed error analysis relevant for implementations based on alkali atom Rydberg states is provided which shows that gate errors less than 10% are possible for k = 35....

Formation of Rydberg states in fast ion-atom collisions

International Nuclear Information System (INIS)

Schneider, D.; Kanter, E.P.; Vager, Z.; Gemmell, D.; Koch, P.; Mariani, D.; Van de Water, W.

1983-01-01

Previous results from beam-foil spectroscopy and from experiments using field ionization techniques have shown that a significant fraction of fast ionic projectiles traversing solid targets can be excited to high Rydberg states. We report an experimental investigation of Rydberg states formed in atomic and molecular ion beams (MeV) emerging from thin-carbon foils. Different field arrangements, including μ-wave fields, have been applied to study the effects of field ionization. The yields of electrons produced via field ionization are compared for different projectile atoms and molecules

Charge-state-distributions of foil-excited heavy Rydberg atoms

International Nuclear Information System (INIS)

Faibis, A.; Kanter, E.P.; Koenig, W.; Zabransky, B.J.

1985-01-01

Studies of foil-excited fast (MeV/amu) heavy ions have demonstrated large yields of high Rydberg atoms formed in such beams. Further experiments have suggested a strong target-thickness dependence of the yields of such atoms. These results have been puzzling in view of the supposed short mean free paths of such atoms in solids. In an effort to better understand these results, the authors have measured the yields of Rydberg atoms (napprox.100-200) in foil-excited 32 S ions at an incident energy of 125 MeV

Autoionizing process of double rydberg states in atom

International Nuclear Information System (INIS)

Xu, X. Y.; Huang, W.; Xu, C. B.; Xue, P.; Chen, D. Y.

1997-01-01

We have studied the autoionization distribution of penetrating double Rydberg (DR) states NLnl(N< n;L,l<4) experimentally in calcium by using five-laser resonance excitation and sequential ionization with a pulsed and a strong constant electric field, as well as theoretically in helium by using the hyperspherical close-coupling method. We have found the DR states autoionize with the ejected electron having its average kinetic energy nearly independent of n but apparently related to the binding energy of the ionic Rydberg orbit NL. We have also discussed the dynamics in DR states and described two types of autoionizing processes, i.e., 'penetration autoionization' and 'polarization autoionization' in DR states

Spin-interaction effects for ultralong-range Rydberg molecules in a magnetic field

Science.gov (United States)

Hummel, Frederic; Fey, Christian; Schmelcher, Peter

2018-04-01

We investigate the fine and spin structure of ultralong-range Rydberg molecules exposed to a homogeneous magnetic field. Each molecule consists of a 87Rb Rydberg atom the outer electron of which interacts via spin-dependent s - and p -wave scattering with a polarizable 87Rb ground-state atom. Our model includes also the hyperfine structure of the ground-state atom as well as spin-orbit couplings of the Rydberg and ground-state atom. We focus on d -Rydberg states and principal quantum numbers n in the vicinity of 40. The electronic structure and vibrational states are determined in the framework of the Born-Oppenheimer approximation for varying field strengths ranging from a few up to hundred Gauss. The results show that the interplay between the scattering interactions and the spin couplings gives rise to a large variety of molecular states in different spin configurations as well as in different spatial arrangements that can be tuned by the magnetic field. This includes relatively regularly shaped energy surfaces in a regime where the Zeeman splitting is large compared to the scattering interaction but small compared to the Rydberg fine structure, as well as more complex structures for both weaker and stronger fields. We quantify the impact of spin couplings by comparing the extended theory to a spin-independent model.

Rabi Oscillations between Ground and Rydberg States with Dipole-Dipole Atomic Interactions

International Nuclear Information System (INIS)

Johnson, T. A.; Urban, E.; Henage, T.; Isenhower, L.; Yavuz, D. D.; Walker, T. G.; Saffman, M.

2008-01-01

We demonstrate Rabi oscillations of small numbers of 87 Rb atoms between ground and Rydberg states with n≤43. Coherent population oscillations are observed for single atoms, while the presence of two or more atoms decoheres the oscillations. We show that these observations are consistent with van der Waals interactions of Rydberg atoms

Evidence of circular Rydberg states in beam-foil experiments: Role of the surface wake field

Science.gov (United States)

Sharma, Gaurav; Puri, Nitin K.; Kumar, Pravin; Nandi, T.

2017-12-01

We have employed the concept of the surface wake field to model the formation of the circular Rydberg states in the beam-foil experiments. The experimental studies of atomic excitation processes show the formation of circular Rydberg states either in the bulk of the foil or at the exit surface, and the mechanism is explained by several controversial theories. The present model is based on the interesting fact that the charge state fraction as well as the surface wake field depend on the foil thickness and it resolves a long-standing discrepancy on the mechanism of the formation of circular Rydberg states. The influence of exit layers is twofold. Initially, the high angular momentum Rydberg states are produced in the last layers of the foil by the Stark switching due to the bulk wake field and finally, they are transferred to the circular Rydberg states as a single multiphoton process due to the influence of the surface wake field.

Photoionization of Rydberg hydrogen atom in a magnetic field

International Nuclear Information System (INIS)

Wang, Dehua; Cheng, Shaohao; Chen, Zhaohang

2015-01-01

Highlights: • The ionization of Rydberg hydrogen atom in a magnetic field has been studied. • Oscillatory structures appear in the electron probability density distributions. • This study can guide the experimental research on the photoionization microscopy. - Abstract: The ionization of Rydberg hydrogen atom in a magnetic field has been studied on the basis of a semiclassical analysis of photoionization microscopy. The photoionization microscopy interference patterns of the photoelectron probability density distribution on a given detector plane are calculated at different scaled energies. We find that due to the interference effect of different types of electron trajectories arrived at a given point on the detector plane, oscillatory structures appear in the electron probability density distributions. The oscillatory structure of the interference pattern, which contains the spatial component of the electronic wave function, evolves sensitively on the scaled energy, through which we gain a deep understanding on the probability density distribution of the electron wave function. This study provides some reference values for the future experiment research on the photoionization microscopy of the Rydberg atom in the presence of magnetic field

Quantum localization in the three-dimensional kicked Rydberg atom

International Nuclear Information System (INIS)

Persson, Emil; Yoshida, Shuhei; Burgdoerfer, Joachim; Tong, X.-M.; Reinhold, Carlos O.

2003-01-01

We study the three-dimensional (3D) unidirectionally kicked Rydberg atom. For parabolic initial states elongated in the direction of the kicks we show that the ionization of the quantum system is suppressed as compared to the classical counterpart and that the quantum wave function is localized along all degrees of freedom, whereas the classical system is globally diffusive. We discuss the connection to the previously studied one-dimensional (1D) model of the kicked Rydberg atom and verify that the 1D model is a good approximation to the 3D quantum case in the limiting case of the most elongated initial states. We further study the quantum phase-space distribution (Husimi distribution) of the eigenstates of the period-one time-evolution (Floquet) operator and show that the eigenstates are localized in phase space. For the most elongated parabolic initial state, we are able to identify the unstable periodic orbits around which Floquet states localize. We discuss the possibility of observing quantum localization in high Rydberg states in n>100

Single-photon cesium Rydberg excitation spectroscopy using 318.6-nm UV laser and room-temperature vapor cell.

Science.gov (United States)

Wang, Jieying; Bai, Jiandong; He, Jun; Wang, Junmin

2017-09-18

We demonstrate a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms in a room-temperature vapor cell. Cs atoms are excited directly from 6S 1/2 ground state to nP 3/2 (n = 70 - 100) Rydberg states with a 318.6 nm ultraviolet (UV) laser, and Rydberg excitation spectra are obtained by transmission enhancement of a probe beam resonant to Cs 6S 1/2 , F = 4 - 6P 3/2 , F' = 5 transition as partial population on F = 4 ground state are transferred to Rydberg state. Analysis reveals that the observed spectra are velocity-selective spectroscopy of Rydberg state, from which the amplitude and linewidth influenced by lasers' Rabi frequency have been investigated. Fitting to energies of Cs nP 3/2 (n = 70 -100) states, the determined quantum defect is 3.56671(42). The demodulated spectra can also be employed as frequency references to stabilize the UV laser frequency to specific Cs Rydberg transition.

Dissipation-induced dipole blockade and antiblockade in driven Rydberg systems

Science.gov (United States)

Young, Jeremy T.; Boulier, Thomas; Magnan, Eric; Goldschmidt, Elizabeth A.; Wilson, Ryan M.; Rolston, Steven L.; Porto, James V.; Gorshkov, Alexey V.

2018-02-01

We study theoretically and experimentally the competing blockade and antiblockade effects induced by spontaneously generated contaminant Rydberg atoms in driven Rydberg systems. These contaminant atoms provide a source of strong dipole-dipole interactions and play a crucial role in the system's behavior. We study this problem theoretically using two different approaches. The first is a cumulant expansion approximation, in which we ignore third-order and higher connected correlations. Using this approach for the case of resonant drive, a many-body blockade radius picture arises, and we find qualitative agreement with previous experimental results. We further predict that as the atomic density is increased, the Rydberg population's dependence on Rabi frequency will transition from quadratic to linear dependence at lower Rabi frequencies. We study this behavior experimentally by observing this crossover at two different atomic densities. We confirm that the larger density system has a smaller crossover Rabi frequency than the smaller density system. The second theoretical approach is a set of phenomenological inhomogeneous rate equations. We compare the results of our rate-equation model to the experimental observations [E. A. Goldschmidt et al., Phys. Rev. Lett. 116, 113001 (2016), 10.1103/PhysRevLett.116.113001] and find that these rate equations provide quantitatively good scaling behavior of the steady-state Rydberg population for both resonant and off-resonant drives.

Quantum-optical magnets with competing short- and long-range interactions: Rydberg-dressed spin lattice in an optical cavity

Directory of Open Access Journals (Sweden)

Jan Gelhausen, Michael Buchhold, Achim Rosch, Philipp Strack

2016-10-01

Full Text Available The fields of quantum simulation with cold atoms [1] and quantum optics [2] are currently being merged. In a set of recent pathbreaking experiments with atoms in optical cavities [3,4] lattice quantum many-body systems with both, a short-range interaction and a strong interaction potential of infinite range -mediated by a quantized optical light field- were realized. A theoretical modelling of these systems faces considerable complexity at the interface of: (i spontaneous symmetry-breaking and emergent phases of interacting many-body systems with a large number of atoms $N\\rightarrow\\infty$, (ii quantum optics and the dynamics of fluctuating light fields, and (iii non-equilibrium physics of driven, open quantum systems. Here we propose what is possibly the simplest, quantum-optical magnet with competing short- and long-range interactions, in which all three elements can be analyzed comprehensively: a Rydberg-dressed spin lattice [5] coherently coupled to a single photon mode. Solving a set of coupled even-odd sublattice Master equations for atomic spin and photon mean-field amplitudes, we find three key results. (R1: Superradiance and a coherent photon field can coexist with spontaneously broken magnetic translation symmetry. The latter is induced by the short-range nearest-neighbor interaction from weakly admixed Rydberg levels. (R2: This broken even-odd sublattice symmetry leaves its imprint in the light via a novel peak in the cavity spectrum beyond the conventional polariton modes. (R3: The combined effect of atomic spontaneous emission, drive, and interactions can lead to phases with anomalous photon number oscillations. Extensions of our work include nano-photonic crystals coupled to interacting atoms and multi-mode photon dynamics in Rydberg systems.

Neutralization of Rubidium Adsorbate Electric Fields by Electron Attachment

Energy Technology Data Exchange (ETDEWEB)

Sedlacek, J. A. [Univ. of Oklahoma, Norman, OK (United States); Kim, E. [Univ. of Nevada, Las Vegas, NV (United States); Rittenhouse, S. T. [Western Washington Univ., Bellingham, WA (United States); US Naval Academy, Annapolis, MD (United States); Weck, Philippe F [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Sadeghpour, H. R. [Harvard-Smithsonian Center for Astrophysics, Cambridge, MA (United States); Shaffer, J. P. [Univ. of Oklahoma, Norman, OK (United States)

2015-10-01

We investigate the (0001) surface of single crystal quartz with a submonolayer of Rb adsorbates. Using Rydberg atom electromagnetically induced transparency, we investigate the electric elds resulting from Rb adsorbed on the quartz surface, and measure the activation energy of the Rb adsorbates. We show that the Rb induces a negative electron affnity (NEA) on the quartz surface. The NEA surface allows for low energy electrons to bind to the surface and cancel the electric eld from the Rb adsorbates. Our results have implications for integrating Rydberg atoms into hybrid quantum systems and the fundamental study of atom-surface interactions, as well as applications for electrons bound to a 2D surface.

Observation of the Borromean Three-Body Förster Resonances for Three Interacting Rb Rydberg Atoms.

Science.gov (United States)

Tretyakov, D B; Beterov, I I; Yakshina, E A; Entin, V M; Ryabtsev, I I; Cheinet, P; Pillet, P

2017-10-27

Three-body Förster resonances at long-range interactions of Rydberg atoms were first predicted and observed in Cs Rydberg atoms by Faoro et al. [Nat. Commun. 6, 8173 (2015)NCAOBW2041-172310.1038/ncomms9173]. In these resonances, one of the atoms carries away an energy excess preventing the two-body resonance, leading thus to a Borromean type of Förster energy transfer. But they were in fact observed as the average signal for the large number of atoms N≫1. In this Letter, we report on the first experimental observation of the three-body Förster resonances 3×nP_{3/2}(|M|)→nS_{1/2}+(n+1)S_{1/2}+nP_{3/2}(|M^{*}|) in a few Rb Rydberg atoms with n=36, 37. We have found here clear evidence that there is no signature of the three-body Förster resonance for exactly two interacting Rydberg atoms, while it is present for N=3-5 atoms. This demonstrates the assumption that three-body resonances can generalize to any Rydberg atom. As such resonance represents an effective three-body operator, it can be used to directly control the three-body interactions in quantum simulations and quantum information processing with Rydberg atoms.

Double sodium rubidium molybdates

International Nuclear Information System (INIS)

Mokhoseev, M.V.; Khal'baeva, K.M.; Khajkina, E.G.; Ogurtsov, A.M.

1990-01-01

According to ceramic technique double sodium-rubidium molybdates of the compositions Rb 2-x Na x MoO 4 (0.5≤x≤0.67) and Na 3 Rb(MoO 4 ) 2 have been prepared. It is ascertained that Rb 2-x Na x MoO 4 is crystallized in glaserite structural type (trigonal crystal system, sp.gr. P3m1, Z=2) and melts incongruently at 640 deg C. Na 3 Rb(MoO 4 ) 2 at room temperature is unstable and gradually decomposes into Na 2 MoO 4 and Rb 2-x Na x MoO 4

Proposal for the determination of nuclear masses by high-precision spectroscopy of Rydberg states

International Nuclear Information System (INIS)

Wundt, B J; Jentschura, U D

2010-01-01

The theoretical treatment of Rydberg states in one-electron ions is facilitated by the virtual absence of the nuclear-size correction, and fundamental constants like the Rydberg constant may be in the reach of planned high-precision spectroscopic experiments. The dominant nuclear effect that shifts transition energies among Rydberg states therefore is due to the nuclear mass. As a consequence, spectroscopic measurements of Rydberg transitions can be used in order to precisely deduce nuclear masses. A possible application of this approach to hydrogen and deuterium, and hydrogen-like lithium and carbon is explored in detail. In order to complete the analysis, numerical and analytic calculations of the quantum electrodynamic self-energy remainder function for states with principal quantum number n = 5, ..., 8 and with angular momentum l = n - 1 and l = n - 2 are described (j = l +- 1/2).

Proposal for the determination of nuclear masses by high-precision spectroscopy of Rydberg states

Energy Technology Data Exchange (ETDEWEB)

Wundt, B J; Jentschura, U D [Department of Physics, Missouri University of Science and Technology, Rolla, MO 65409-0640 (United States)

2010-06-14

The theoretical treatment of Rydberg states in one-electron ions is facilitated by the virtual absence of the nuclear-size correction, and fundamental constants like the Rydberg constant may be in the reach of planned high-precision spectroscopic experiments. The dominant nuclear effect that shifts transition energies among Rydberg states therefore is due to the nuclear mass. As a consequence, spectroscopic measurements of Rydberg transitions can be used in order to precisely deduce nuclear masses. A possible application of this approach to hydrogen and deuterium, and hydrogen-like lithium and carbon is explored in detail. In order to complete the analysis, numerical and analytic calculations of the quantum electrodynamic self-energy remainder function for states with principal quantum number n = 5, ..., 8 and with angular momentum l = n - 1 and l = n - 2 are described (j = l {+-} 1/2).

Rubidium selenatoindiates

International Nuclear Information System (INIS)

Kadoshnikova, N.V.; Dejchman, Eh.N.; Tananaev, I.V.

1977-01-01

Interaction of aqueous solutions of indium and rubidium selenates at 20 deg C has been investigated. From the experimental data obtained in studying solubility in the Rb 2 SeO 4 -In 2 (SeO 4 ) 3 -H 2 O system it follows that at n=[Rb 2 SeO 4 ]/[In 2 SeO 4 ) 3 ]( 4 ) 2 x4H 2 O is formed. The optimum conditions for obtaining this product are solutions with n=3-5 at increased acidity (approximately 5%H 2 SeO 4 ). RbIn(SeO 4 ) 2 x4H 2 O consists of negative biaxial crystals. Dehydration occurs in a single stage. The substance obtained is hydrolized in excess Rb 2 SO 4 with the formation of basic salts of variable composition. RbIn(SeO 4 ) 2 x4H 2 O has been investigated crystal-optically, thermographically, and roentgenographically

Interaction of K(nd) Rydberg atoms with an amorphous gold surface

International Nuclear Information System (INIS)

Gray, D.F.

1988-01-01

This thesis reports the first controlled study of the interactions of Rydberg atoms with a metal surface. In these experiments, a collimated beam of potassium Rydberg atoms is directed at a plane surface at near grazing incidence. Positive ions formed by surface ionization are attracted to the surface by their image charge, which is counterbalanced by an external electric field applied perpendicular to the surface. The ions are detected by a position-sensitive detector (PSD). At some critical value of the external field, the ion trajectories just miss the surface, suggesting that analysis of the dependence of the ion signals of external electric field can be used to determine the distance from the surface at which ionization occurs. This distance, and thus the corresponding critical electric field, is expected to be n-dependent. Experimentally, however, it was observed that the ion signal had a sudden n-independent onset when only a small positive perpendicular electric field was applied at the surface. This observation requires, surprisingly, that the ions produced by surface ionization can readily escape from the surface. The data do, however, show that Rydberg atoms are efficiently ionized in collisions with the surface. This process may provide a useful new detection technique for Rydberg atoms

A gravimetric and an X-ray fluorescence method for the determination of rubidium in Rb2U(SO4)3

International Nuclear Information System (INIS)

Mudher, K.D.S.; Krishnan, K.; Jayadevan, N.C.

1993-01-01

Chemical characterization of rubidium uranium(IV) trisulfate, RB 2 U(SO 4 ) 3 , a new chemical assay standard for uranium requires accurate analysis of rubidium. A gravimetric and an X-ray fluorescence method (XRF) for the determination of rubidium in this compound are described. In the gravimetric method, rubidium is determined as Rb 2 Na[Co(NO 2 ) 6 ].H 2 O without separating uranium with a precision of the order of ±0.5%. In the XRF method, the concentration ratio of rubidium to uranium, C Rb /C U , is determined in the solid samples by the binary ratio method using calibration between intensity ratios (I Rb /I U ) and concentration ratios (C Rb /C U ). (author) 6 refs.; 2 figs.; 3 tabs

Rydberg excitation of neutral nitric oxide molecules in strong UV and near-IR laser fields

International Nuclear Information System (INIS)

Lv Hang; Zhang Jun-Feng; Zuo Wan-Long; Xu Hai-Feng; Jin Ming-Xing; Ding Da-Jun

2015-01-01

Rydberg state excitations of neutral nitric oxide molecules are studied in strong ultraviolet (UV) and near-infra-red (IR) laser fields using a linear time-of-flight (TOF) mass spectrometer with the pulsed electronic field ionization method. The yield of Rydberg molecules is measured as a function of laser intensity and ellipticity, and the results in UV laser fields are compared with those in near-IR laser fields. The present study provides the first experimental evidence of neutral Rydberg molecules surviving in a strong laser field. The results indicate that a rescattering-after-tunneling process is the main contribution to the formation of Rydberg molecules in strong near-IR laser fields, while multi-photon excitation may play an important role in the strong UV laser fields. (paper)

Asymptomatic myocardial ischemia following cold provocation

International Nuclear Information System (INIS)

Shea, M.J.; Deanfield, J.E.; deLandsheere, C.M.; Wilson, R.A.; Kensett, M.; Selwyn, A.P.

1987-01-01

Cold is thought to provoke angina in patients with coronary disease either by an increase in myocardial demand or an increase in coronary vascular resistance. We investigated and compared the effects of cold pressor stimulation and symptom-limited supine bicycle exercise on regional myocardial perfusion in 35 patients with stable angina and coronary disease and in 10 normal subjects. Regional myocardial perfusion was assessed with positron emission tomography and rubidium-82. Following cold pressor stimulation 24 of 35 patients demonstrated significant abnormalities of regional myocardial perfusion with reduced cation uptake in affected regions of myocardium: 52 +/- 9 to 43 +/- 9 (p less than 0.001 vs normal subjects). Among these 24 patients only nine developed ST depression and only seven had angina. In contrast, 29 of 35 patients underwent supine exercise, and abnormal regional myocardial perfusion occurred in all 29, with a reduction in cation intake from 48 +/- 10 to 43 +/- 14 (p less than 0.001 vs normal subjects). Angina was present in 27 of 29 and ST depression in 25 of 29. Although the absolute decrease in cation uptake was somewhat greater following cold as opposed to exercise, the peak heart rate after cold was significantly lower than that after exercise (82 +/- 12 vs 108 +/- 16 bpm, p less than 0.05). Peak systolic blood pressures after cold and exercise were similar (159 +/- 24 vs 158 +/- 28). Thus, cold produces much more frequent asymptomatic disturbances of regional myocardial perfusion in patients with stable angina and coronary disease than is suggested by pain or ECG changes

Application of the Faddeev-Watson expansion to thermal collisions of Rydberg atoms with neutral particles

International Nuclear Information System (INIS)

de Prunele, E.

1983-01-01

The Faddeev-Watson expansion (FWE) for the T operator is applied to the study of thermal collisions between Rydberg atom and neutral atom. These collisions are considered as a three-body problem (the perturber, the Rydberg electron, and its parent core) and it is assumed, as already done in most theoretical works dealing with Rydberg-atom--atom collisions, that the core-perturber interaction can be neglected. Then the evaluation of the FWE first- and second-order terms is made tractable by using an appropriate separable potential for the Rydberg-electron--perturber interaction. The evaluation of the second-order term allows us to estimate the importance of taking into account explicitly the Rydberg-electron--core interaction in the expression of the (three-body) T operator for the thermal collisions considered. Detailed calculations for the process Rb(n, l = 0)+He →Rb(n',l')+He are presented and discussed. The FWE second-order term has been evaluated for the first time by taking the (two-body) t operator associated with the Rydberg atom (valence electron plus parent core) as the Coulomb potential. The contribution of the FWE second-order term to the scattering amplitude decreases as n increases and is found especially significant when both the momentum transfers involved in the collision are large and the values of l and l' are small

Rydberg states of chloroform studied by VUV photoabsorption spectroscopy

International Nuclear Information System (INIS)

Singh, Param Jeet; Shastri, Aparna; D’Souza, R.; Jagatap, B.N.

2013-01-01

The VUV photoabsorption spectra of CHCl 3 and CDCl 3 in the energy region 6.2–11.8 eV (50,000–95,000 cm −1 ) have been investigated using synchrotron radiation from the Indus-1 source. Rydberg series converging to the first four ionization limits at 11.48, 11.91, 12.01 and 12.85 eV corresponding to excitation from the 1a 2 , 4a 1 , 4e, 3e, orbitals of CHCl 3 respectively are identified and analyzed. Quantum defect values are observed to be consistent with excitation from the chlorine lone pair orbitals. Vibrational progressions observed in the region of 72,500–76,500 cm −1 have been reassigned to ν 3 and combination modes of ν 3 +ν 6 belonging to the 1a 2 →4p transition in contrast to earlier studies where they were assigned to a ν 3 progression superimposed on the 3e→4p Rydberg transition. The assignments are further confirmed based on isotopic substitution studies on CDCl 3 whose VUV photoabsorption spectrum is reported here for the first time. The frequencies of the ν 3 and ν 6 modes in the 4p Rydberg state of CHCl 3 (CDCl 3 ) are proposed to be ∼454 (409) cm −1 and∼130 (129) cm −1 respectively based on the vibronic analysis. DFT calculations of neutral and ionic ground state vibrational frequencies support the vibronic analysis. Experimental spectrum is found to be in good agreement with that predicted by TDDFT calculations. This work presents a consolidated analysis of the VUV photoabsorption spectrum of chloroform. -- Highlights: •VUV photoabsorption spectra of CHCl 3 and CDCl 3 studied using synchrotron radiation. •Quantum defect analysis of Rydberg series converging to first four ionization limits. •Vibronic bands in 72,500–76,500 cm −1 region assigned to 1a 2 →4p Rydberg transition. •Vibrational progressions assigned to ν 3 and ν 3 +ν 6 using ab initio calculations. •Excellent agreement of TDDFT vertical excited energies with experimental spectrum

Analysis of imperfections in the coherent optical excitation of single atoms to Rydberg states

Science.gov (United States)

de Léséleuc, Sylvain; Barredo, Daniel; Lienhard, Vincent; Browaeys, Antoine; Lahaye, Thierry

2018-05-01

We study experimentally various physical limitations and technical imperfections that lead to damping and finite contrast of optically driven Rabi oscillations between ground and Rydberg states of a single atom. Finite contrast is due to preparation and detection errors, and we show how to model and measure them accurately. Part of these errors originates from the finite lifetime of Rydberg states, and we observe its n3 scaling with the principal quantum number n . To explain the damping of Rabi oscillations, we use simple numerical models taking into account independently measured experimental imperfections and show that the observed damping actually results from the accumulation of several small effects, each at the level of a few percent. We discuss prospects for improving the coherence of ground-Rydberg Rabi oscillations in view of applications in quantum simulation and quantum information processing with arrays of single Rydberg atoms.

Wave packet fractional revivals in a one-dimensional Rydberg atom

International Nuclear Information System (INIS)

Veilande, Rita; Bersons, Imants

2007-01-01

We investigate many characteristic features of revival and fractional revival phenomena via derived analytic expressions for an autocorrelation function of a one-dimensional Rydberg atom with weighting probabilities modelled by a Gaussian or a Lorentzian distribution. The fractional revival phenomenon in the ionization probabilities of a one-dimensional Rydberg atom irradiated by two short half-cycle pulses is also studied. When many states are involved in the formation of the wave packet, the revival is lower and broader than the initial wave packet and the fractional revivals overlap and disappear with time

Many-body dynamics of driven-dissipative Rydberg cavity polaritons

Science.gov (United States)

Pistorius, Tim; Fan, Jingtao; Weimer, Hendrik

2017-04-01

The usage of photons as long-range information carriers has greatly increased the interest in systems with nonlinear optical properties in recent years. The nonlinearity is easily achievable in Rydberg mediums through the strong van der Waals interaction which makes them one of the best candidates for such a system. Here, we propose a way to analyze the steady state solutions of a Rydberg medium in a cavity through the combination of the variational principle for open quantum systems and the P-distribution of the density matrix. To get a better understanding of the many-body-dynamics a transformation into the polariton picture is performed and investigated. Volkswagen Foundation, Deutsche Forschungsgemeinschaft.

Evolution from Rydberg gas to ultracold plasma in a supersonic atomic beam of Xe

International Nuclear Information System (INIS)

Hung, J; Sadeghi, H; Schulz-Weiling, M; Grant, E R

2014-01-01

A Rydberg gas of xenon, entrained in a supersonic atomic beam, evolves slowly to form an ultracold plasma. In the early stages of this evolution, when the free-electron density is low, Rydberg atoms undergo long-range ℓ-mixing collisions, yielding states of high orbital angular momentum. The development of high-ℓ states promotes dipole–dipole interactions that help to drive Penning ionization. The electron density increases until it reaches the threshold for avalanche. Ninety μs after the production of a Rydberg gas with the initial state, n 0 ℓ 0 =42d, a 432 V cm −1 electrostatic pulse fails to separate charge in the excited volume, an effect which is ascribed to screening by free electrons. Photoexcitation cross sections, observed rates of ℓ-mixing, and a coupled-rate-equation model simulating the onset of the electron-impact avalanche point consistently to an initial Rydberg gas density of 5×10 8 cm −3 . (paper)

Evolution from Rydberg gas to ultracold plasma in a supersonic atomic beam of Xe

Science.gov (United States)

Hung, J.; Sadeghi, H.; Schulz-Weiling, M.; Grant, E. R.

2014-08-01

A Rydberg gas of xenon, entrained in a supersonic atomic beam, evolves slowly to form an ultracold plasma. In the early stages of this evolution, when the free-electron density is low, Rydberg atoms undergo long-range \\ell -mixing collisions, yielding states of high orbital angular momentum. The development of high-\\ell states promotes dipole-dipole interactions that help to drive Penning ionization. The electron density increases until it reaches the threshold for avalanche. Ninety μs after the production of a Rydberg gas with the initial state, {{n}_{0}}{{\\ell }_{0}}=42d, a 432 V cm-1 electrostatic pulse fails to separate charge in the excited volume, an effect which is ascribed to screening by free electrons. Photoexcitation cross sections, observed rates of \\ell -mixing, and a coupled-rate-equation model simulating the onset of the electron-impact avalanche point consistently to an initial Rydberg gas density of 5\\times {{10}^{8}}\\;c{{m}^{-3}}.

82 Rubidium-PET kan blive den nye myokardieskintigrafi

DEFF Research Database (Denmark)

Hasbak, Philip; Kjær, Andreas

2011-01-01

-lived isotopes at centres with access to a cyclotron, and only including a very limited number of patients. The number of PET scanners has increased markedly in Denmark and with the introduction of generator-produced 82-Rubidium, this modality may replace the traditional cardial single photon emission computed...

High Angular Momentum Rydberg Wave Packets

Science.gov (United States)

Wyker, Brendan

2011-12-01

High angular momentum Rydberg wave packets are studied. Application of carefully tailored electric fields to low angular momentum, high- n (n ˜ 300) Rydberg atoms creates coherent superpositions of Stark states with near extreme values of angular momentum, ℓ. Wave packet components orbit the parent nucleus at rates that depend on their energy, leading to periods of localization and delocalization as the components come into and go out of phase with each other. Monitoring survival probability signals in the presence of position dependent probing leads to observation of characteristic oscillations based on the composition of the wave packet. The discrete nature of electron energy levels is observed through the measurement of quantum revivals in the wave packet localization signal. Time-domain spectroscopy of these signals allows determination of both the population and phase of individual superposition components. Precise manipulation of wave packets is achieved through further application of pulsed electric fields. Decoherence effects due to background gas collisions and electrical noise are also detailed. Quantized classical trajectory Monte-Carlo simulations are introduced and agree remarkably well with experimental results.

Fundamental constants and tests of theory in Rydberg states of hydrogenlike ions.

Science.gov (United States)

Jentschura, Ulrich D; Mohr, Peter J; Tan, Joseph N; Wundt, Benedikt J

2008-04-25

A comparison of precision frequency measurements to quantum electrodynamics (QED) predictions for Rydberg states of hydrogenlike ions can yield information on values of fundamental constants and test theory. With the results of a calculation of a key QED contribution reported here, the uncertainty in the theory of the energy levels is reduced to a level where such a comparison can yield an improved value of the Rydberg constant.

Fundamental Constants and Tests of Theory in Rydberg States of Hydrogenlike Ions

International Nuclear Information System (INIS)

Jentschura, Ulrich D.; Mohr, Peter J.; Tan, Joseph N.; Wundt, Benedikt J.

2008-01-01

A comparison of precision frequency measurements to quantum electrodynamics (QED) predictions for Rydberg states of hydrogenlike ions can yield information on values of fundamental constants and test theory. With the results of a calculation of a key QED contribution reported here, the uncertainty in the theory of the energy levels is reduced to a level where such a comparison can yield an improved value of the Rydberg constant

Ionization of Rb Rydberg atoms in the attractive nsnp dipole-dipole potential

International Nuclear Information System (INIS)

Park, Hyunwook; Shuman, E. S.; Gallagher, T. F.

2011-01-01

We have observed the ionization of a cold gas of Rb Rydberg atoms which occurs when nsns van der Waals pairs of ns atoms of n≅ 40 on a weakly repulsive potential are transferred to an attractive dipole-dipole nsnp potential by a microwave transition. Comparing the measurements to a simple model shows that the initial 300-μK thermal velocity of the atoms plays an important role. Excitation to a repulsive dipole-dipole potential does not lead to more ionization on a 15-μs time scale than leaving the atoms in the weakly repulsive nsns state. This observation is slightly surprising since a radiative transition must occur to allow ionization in the latter case. Finally, by power broadening of the microwave transition, to allow transitions from the initial nsns state to the nsnp state over a broad range of internuclear spacings, it is possible to accelerate markedly the evolution to a plasma.

Entropy and complexity analysis of hydrogenic Rydberg atoms

Energy Technology Data Exchange (ETDEWEB)

Lopez-Rosa, S. [Instituto Carlos I de Fisica Teorica y Computacional, Universidad de Granada, 18071-Granada (Spain); Departamento de Fisica Aplicada II, Universidad de Sevilla, 41012-Sevilla (Spain); Toranzo, I. V.; Dehesa, J. S. [Instituto Carlos I de Fisica Teorica y Computacional, Universidad de Granada, 18071-Granada (Spain); Departamento de Fisica Atomica, Molecular y Nuclear, Universidad de Granada, 18071-Granada (Spain); Sanchez-Moreno, P. [Instituto Carlos I de Fisica Teorica y Computacional, Universidad de Granada, 18071-Granada (Spain); Departamento de Matematica Aplicada, Universidad de Granada, 18071-Granada (Spain)

2013-05-15

The internal disorder of hydrogenic Rydberg atoms as contained in their position and momentum probability densities is examined by means of the following information-theoretic spreading quantities: the radial and logarithmic expectation values, the Shannon entropy, and the Fisher information. As well, the complexity measures of Cramer-Rao, Fisher-Shannon, and Lopez Ruiz-Mancini-Calvet types are investigated in both reciprocal spaces. The leading term of these quantities is rigorously calculated by use of the asymptotic properties of the concomitant entropic functionals of the Laguerre and Gegenbauer orthogonal polynomials which control the wavefunctions of the Rydberg states in both position and momentum spaces. The associated generalized Heisenberg-like, logarithmic and entropic uncertainty relations are also given. Finally, application to linear (l= 0), circular (l=n- 1), and quasicircular (l=n- 2) states is explicitly done.

Molecular ions, Rydberg spectroscopy and dynamics

International Nuclear Information System (INIS)

Jungen, Ch.

2015-01-01

Ion spectroscopy, Rydberg spectroscopy and molecular dynamics are closely related subjects. Multichannel quantum defect theory is a theoretical approach which draws on this close relationship and thereby becomes a powerful tool for the study of systems consisting of a positively charged molecular ion core interacting with an electron which may be loosely bound or freely scattering

Molecular ions, Rydberg spectroscopy and dynamics

Energy Technology Data Exchange (ETDEWEB)

Jungen, Ch. [Laboratoire Aimé Cotton, Université de Paris-Sud, 91405 Orsay (France)

2015-01-22

Ion spectroscopy, Rydberg spectroscopy and molecular dynamics are closely related subjects. Multichannel quantum defect theory is a theoretical approach which draws on this close relationship and thereby becomes a powerful tool for the study of systems consisting of a positively charged molecular ion core interacting with an electron which may be loosely bound or freely scattering.

Nuclear spin transitions in the kHz range in Rydberg matter clusters give precise values of the internal magnetic field from orbiting Rydberg electrons

International Nuclear Information System (INIS)

Holmlid, Leif

2009-01-01

Clusters of the electronically excited condensed matter Rydberg matter (RM) are planar and sixfold symmetric with specific magic numbers N as shown by rotational spectroscopy of potassium K N clusters [L. Holmlid, Mol. Phys. 105 (2007) 933; L. Holmlid, J. Mol. Struct. 885 (2008) 122]. In radio frequency emission spectra from such clusters, features are observed that are due to the hyperfine interaction between the atomic nucleus 39 K and two Rydberg electrons. These electrons exist in a doubly excited K atom at n'' = 5 or 6 in a 'sleeping-top' type rotating cluster. Such low excited electrons were observed recently in optical intra-cavity experiments in K(RM), where the electrons in the conduction band are involved in the angular momentum conservation in the stimulated emission. Here we show that the agreement with the theoretical description of circular Rydberg states is excellent within ±0.2% in the magnetic field, invoking angular momentum conservation by electrons in the condensed phase. Sleeping-top clusters may form stacks of clusters, and it is likely that such stacks are the emitting entities involved in the two nuclear spin series observed.

Combined theoretical and experimental study of the valence, Rydberg and ionic states of fluorobenzene

Energy Technology Data Exchange (ETDEWEB)

Palmer, Michael H., E-mail: m.h.palmer@ed.ac.uk; Ridley, Trevor [School of Chemistry, University of Edinburgh, Joseph Black Building, David Brewster Road, Edinburgh, Scotland EH9 3FJ (United Kingdom); Vrønning Hoffmann, Søren, E-mail: vronning@phys.au.dk, E-mail: nykj@phys.au.dk, E-mail: marcello.coreno@elettra.eu, E-mail: desimone@iom.cnr.it, E-mail: Teng.Zhang@physics.uu.se, E-mail: biczysko@shu.edu.cn, E-mail: alberto.baiardi@sns.it, E-mail: kipeters@wsu.edu; Jones, Nykola C., E-mail: vronning@phys.au.dk, E-mail: nykj@phys.au.dk, E-mail: marcello.coreno@elettra.eu, E-mail: desimone@iom.cnr.it, E-mail: Teng.Zhang@physics.uu.se, E-mail: biczysko@shu.edu.cn, E-mail: alberto.baiardi@sns.it, E-mail: kipeters@wsu.edu [ISA, Department of Physics and Astronomy, Aarhus University, Ny Munkegade 120, DK-8000 Aarhus C (Denmark); Coreno, Marcello, E-mail: vronning@phys.au.dk, E-mail: nykj@phys.au.dk, E-mail: marcello.coreno@elettra.eu, E-mail: desimone@iom.cnr.it, E-mail: Teng.Zhang@physics.uu.se, E-mail: biczysko@shu.edu.cn, E-mail: alberto.baiardi@sns.it, E-mail: kipeters@wsu.edu [CNR-ISM, Basovizza Area Science Park, 1-34149 Trieste (Italy); De Simone, Monica, E-mail: vronning@phys.au.dk, E-mail: nykj@phys.au.dk, E-mail: marcello.coreno@elettra.eu, E-mail: desimone@iom.cnr.it, E-mail: Teng.Zhang@physics.uu.se, E-mail: biczysko@shu.edu.cn, E-mail: alberto.baiardi@sns.it, E-mail: kipeters@wsu.edu [CNR-IOM Laboratorio TASC, Trieste (Italy); Grazioli, Cesare [CNR-IOM Laboratorio TASC, Trieste (Italy); Department of Chemical and Pharmaceutical Sciences, University of Trieste, Trieste (Italy); Zhang, Teng, E-mail: vronning@phys.au.dk, E-mail: nykj@phys.au.dk, E-mail: marcello.coreno@elettra.eu, E-mail: desimone@iom.cnr.it, E-mail: Teng.Zhang@physics.uu.se, E-mail: biczysko@shu.edu.cn, E-mail: alberto.baiardi@sns.it, E-mail: kipeters@wsu.edu [Department of Physics and Astronomy, University of Uppsala, Uppsala (Sweden); and others

2016-05-28

New photoelectron spectra (PES) and ultra violet (UV) and vacuum UV (VUV) absorption spectra of fluorobenzene recorded at higher resolution than previously, have been combined with mass-resolved (2 + 1) and (3 + 1) resonance enhanced multiphoton ionization (REMPI) spectra; this has led to the identification of numerous Rydberg states. The PES have been compared with earlier mass-analyzed threshold ionization and photoinduced Rydberg ionization (PIRI) spectra to give an overall picture of the ionic state sequence. The analysis of these spectra using both equations of motion with coupled cluster singles and doubles (EOM-CCSD) configuration interaction and time dependent density functional theory (TDDFT) calculations have been combined with vibrational analysis of both the hot and cold bands of the spectra, in considerable detail. The results extend several earlier studies on the vibronic coupling leading to conical intersections between the X{sup 2}B{sub 1} and A{sup 2}A{sub 2} states, and a further trio (B, C, and D) of states. The conical intersection of the X and A states has been explicitly identified, and its structure and energetics evaluated. The energy sequence of the last group is only acceptable to the present study if given as B{sup 2}B{sub 2}

Heavy Rydberg behaviour in high vibrational levels of some ion-pair states of the halogens and inter-halogens

International Nuclear Information System (INIS)

Donovan, Robert J.; Lawley, Kenneth P.; Ridley, Trevor

2015-01-01

We report the identification of heavy Rydberg resonances in the ion-pair spectra of I 2 , Cl 2 , ICl, and IBr. Extensive vibrational progressions are analysed in terms of the energy dependence of the quantum defect δ(E b ) rather than as Dunham expansions. This is shown to define the heavy Rydberg region, providing a more revealing fit to the data with fewer coefficients and leads just as easily to numbering data sets separated by gaps in the observed vibrational progressions. Interaction of heavy Rydberg states with electronic Rydberg states at avoided crossings on the inner wall of the ion-pair potential is shown to produce distinctive changes in the energy dependence of δ(E b ), with weak and strong interactions readily distinguished. Heavy Rydberg behaviour is found to extend well below near-dissociation states, down to vibrational levels ∼18 000-20 000 cm −1 below dissociation. The rapid semi-classical calculation of δ(E b ) for heavy Rydberg states is emphasised and shows their absolute magnitude to be essentially the volume of phase space excluded from the vibrational motion by avoiding core-core penetration of the ions

Orbital alignment effects in near-resonant Rydberg atoms-rare gas collisions

International Nuclear Information System (INIS)

Isaacs, W.A.; Morrison, M.A.

1993-01-01

Recent experimental and theoretical studies of near-resonant energy transfer collisions involving rare-gas atoms and alkali or alkaline earth atoms which have been initially excited to an aligned state via one or more linearly polarized rasters have yielded a wealth of insight into orbital alignment and related effects. We have extended this inquiry to initially aligned Rydberg states, examining state-to-state and alignment-selected cross sections using quantum collision theory augmented by approximations appropriate to the special characteristics of the Rydberg state (e.g., the quasi-free-electron model and the impulse approximation)

Effect of finite detection efficiency on the observation of the dipole-dipole interaction of a few Rydberg atoms

International Nuclear Information System (INIS)

Ryabtsev, I. I.; Tretyakov, D. B.; Beterov, I. I.; Entin, V. M.

2007-01-01

We have developed a simple analytical model describing multiatom signals that are measured in experiments on dipole-dipole interaction at resonant collisions of a few Rydberg atoms. It has been shown that finite efficiency of the selective field-ionization detector leads to the mixing up of the spectra of resonant collisions registered for various numbers of Rydberg atoms. The formulas which help to estimate an appropriate mean Rydberg atom number for a given detection efficiency are presented. We have found that a measurement of the relation between the amplitudes of collisional resonances observed in the one- and two-atom signals provides a straightforward determination of the absolute detection efficiency and mean Rydberg atom number. We also performed a testing experiment on resonant collisions in a small excitation volume of a sodium atomic beam. The resonances observed for 1-4 detected Rydberg atoms have been analyzed and compared with theory

Rubidium-strontium and uranium-lead isotopic age studies

International Nuclear Information System (INIS)

Loveridge, W.D.

1980-01-01

Rubidium-strontium whole rock isochron ages and initial 87 Sr/ 86 Sr ratios and uranium-lead ages on zircon from suites of samples selected from localities across Canada are presented. Descriptions of the geological probelms and interpretations of the measured ages are included. Laboratory age determination methods and techniques are described or referenced. (auth)

Entropy and complexity analysis of hydrogenic Rydberg atoms

International Nuclear Information System (INIS)

López-Rosa, S.; Toranzo, I. V.; Dehesa, J. S.; Sánchez-Moreno, P.

2013-01-01

The internal disorder of hydrogenic Rydberg atoms as contained in their position and momentum probability densities is examined by means of the following information-theoretic spreading quantities: the radial and logarithmic expectation values, the Shannon entropy, and the Fisher information. As well, the complexity measures of Crámer-Rao, Fisher-Shannon, and López Ruiz-Mancini-Calvet types are investigated in both reciprocal spaces. The leading term of these quantities is rigorously calculated by use of the asymptotic properties of the concomitant entropic functionals of the Laguerre and Gegenbauer orthogonal polynomials which control the wavefunctions of the Rydberg states in both position and momentum spaces. The associated generalized Heisenberg-like, logarithmic and entropic uncertainty relations are also given. Finally, application to linear (l= 0), circular (l=n− 1), and quasicircular (l=n− 2) states is explicitly done.

Determination of first ionization potential of samarium atom using Rydberg series convergence

International Nuclear Information System (INIS)

Jayasekharan, T.; Razvi, M.A.N.; Bhale, G.L.

1999-01-01

The study of Rydberg states has recently received more attention partially because an efficient isotope selective ionization is possible via these states. In addition, their investigation provides useful information on the atomic structure. An electron in a shell with a high principal quantum number is a sensitive probe for the interaction with the ionic core of the atom. Measurements of these Rydberg levels give valuable data on quantum defects, anomalies in fine structure splitting, polarizabilities, configuration interactions, ionization potentials etc

From the Rydberg constant to the fundamental constants metrology; De la constante de Rydberg a la metrologie des constantes fondamentales

Energy Technology Data Exchange (ETDEWEB)

Nez, F

2005-06-15

This document reviews the theoretical and experimental achievements of the author since the beginning of his scientific career. This document is dedicated to the spectroscopy of hydrogen, deuterium and helium atoms. The first part is divided into 6 sub-sections: 1) the principles of hydrogen spectroscopy, 2) the measurement of the 2S-nS/nD transitions, 3) other optical frequency measurements, 4) our contribution to the determination of the Rydberg constant, 5) our current experiment on the 1S-3S transition, 6) the spectroscopy of the muonic hydrogen. Our experiments have improved the accuracy of the Rydberg Constant by a factor 25 in 15 years and we have achieved the first absolute optical frequency measurement of a transition in hydrogen. The second part is dedicated to the measurement of the fine structure constant and the last part deals with helium spectroscopy and the search for optical references in the near infrared range. (A.C.)

Isotopic rubidium ion efflux assay for the functional characterization of nicotinic acetylcholine receptors on clonal cell lines

International Nuclear Information System (INIS)

Lukas, R.J.; Cullen, M.J.

1988-01-01

An isotopic rubidium ion efflux assay has been developed for the functional characterization of nicotinic acetylcholine receptors on cultured neurons. This assay first involves the intracellular sequestration of isotopic potassium ion analog by the ouabain-sensitive action of a sodium-potassium ATPase. Subsequently, the release of isotopic rubidium ion through nicotinic acetylcholine receptor-coupled monovalent cation channels is activated by application of nicotinic agonists. Specificity of receptor-mediated efflux is demonstrated by its sensitivity to blockade by nicotinic, but not muscarinic, antagonists. The time course of agonist-mediated efflux, within the temporal limitations of the assay, indicates a slow inactivation of receptor function on prolonged exposure to agonist. Dose-response profiles (i) have characteristic shapes for different nicotinic agonists, (ii) are described by three operationally defined parameters, and (iii) reflect different affinities of agonists for binding sites that control receptor activation and functional inhibition. The rubidium ion efflux assay provides fewer hazards but greater sensitivity and resolution than isotopic sodium or rubidium ion influx assays for functional nicotinic receptors

Control of the 133 cesium cold collisions, search for a variation of the fine structure constant using a dual rubidium-cesium atomic fountain

International Nuclear Information System (INIS)

Marion, H.

2005-03-01

We developed a method of measurement of the frequency shift due to the collisions between cold atoms. This is the main systematic limitation for the accuracy of the Cs 133 based fountains (∼ 10 -15 in relative frequency). Consequently, we can measure this effect near 0.5% This opens prospects for improvements of the fountains performances in term of accuracy until 10 -16 . The fountain has also obtained a stability about 10 -14 at 1 s. We discovered for the first time, at very low magnetic field (5 ± 1 mG), Feshbach resonances. We also took a new absolute measurement of the hyperfine transition of the Rb 87 , which is the most precise ever carried out and is used now as definition for the secondary standard. By comparing this value with those measured the previous years, we could carry out a test of the stability of the fine structure constant on the level of 10 -15 /yr. We led local comparisons between atomic fountains and the other fountains of the laboratory. Most stable it is unrolled with a combined stability of 5.10 -14 at 1 s. The behavior of the difference of the two clocks goes like white frequency noise up to 3.10 -16 . The assessment of the dual fountain accuracy budget has been evaluated at 7.10 -16 for the cesium part and 8.10 -16 for the rubidium part. We contributed to the realization of the scale of International Atomic Time, by series of calibrations of hydrogen masers. An atomic comparison of fountain by satellite links was tested between our laboratory and our German counterpart. This measurement has determined the good agreement between the two clocks. (author)

Fermionic Collective Excitations in a Lattice Gas of Rydberg Atoms

International Nuclear Information System (INIS)

Olmos, B.; Gonzalez-Ferez, R.; Lesanovsky, I.

2009-01-01

We investigate the many-body quantum states of a laser-driven gas of Rydberg atoms confined to a large spacing ring lattice. If the laser driving is much stronger than the van der Waals interaction among the Rydberg atoms, these many-body states are collective fermionic excitations. The first excited state is a spin wave that extends over the entire lattice. We demonstrate that our system permits us to study fermions in the presence of disorder although no external atomic motion takes place. We analyze how this disorder influences the excitation properties of the fermionic states. Our work shows a route towards the creation of complex many-particle states with atoms in lattices.

Interstellar Lithium and Rubidium in the Diffuse Gas Near IC 443

Science.gov (United States)

Ritchey, Adam M.; Taylor, C. J.; Federman, S. R.; Lambert, D. L.

2011-01-01

We present an analysis of interstellar lithium and rubidium from observations made with the Hobby-Eberly Telescope at McDonald Observatory of the Li I λ6707 and Rb I λ7800 absorption lines along four lines of sight through the supernova remnant IC 443. The observations probe interstellar material polluted by the ejecta of a core-collapse (Type II) supernova and can thus be used to constrain the contribution from massive stars to the synthesis of lithium and rubidium. Production of 7Li is expected to occur through neutrino spallation in the helium and carbon shells of the progenitor star during the terminal supernova explosion, while both 6Li and 7Li are synthesized via spallation and fusion reactions involving cosmic rays accelerated by the remnant. Gamma-ray emission from IC 443 provides strong evidence for the interaction of accelerated cosmic rays with the ambient atomic and molecular gas. Rubidium is also produced by massive stars through the weak s-process in the He- and C-burning shells and the r-process during core collapse. We examine interstellar 7Li/6Li isotope ratios as well as Li/K and Rb/K ratios along each line of sight, and discuss the implications of our results in the context of nucleosynthesis associated with Type II supernovae.

Investigation by high resolution electron spectroscopy of the helium-like 3lnl' Rydberg series in double capture processes at low collision velocity: auto transfer to Rydberg states and electron stabilization

International Nuclear Information System (INIS)

Bordenave-Montesquieu, A.; Moretto-Capelle, P.; Gonzalez, A.; Benhenni, M.; Bachau, H.; Sanchez, I.

1994-01-01

A high resolution electron spectrometry of the (3lnl') Ryberg series populated in N 7+ + He and Ne 10+ + He collisions at 10 q keV, 10 o allows us to observe, for the first time by this method, two post-collisional effects. First, it is found with nitrogen ions that, when n increases from n = 4 to 9, the L-distribution peaks more and more on the high angular momentum states. This is qualitatively understood as a Stark deformation of the Rydberg orbit by the Coulomb field of the receding ion. Also, in the n range where the double capture process populates symmetrical 4l4l' states (n>9), an enhancement of the intensities of the 3lnl' Rydberg lines is observed for both collisonal systems. This is thought to be a signature of the so-called auto transfer to Rydberg states effect. The transfer of population from the 3l4l' to the 3lnl' states is found to be favoured against a direct autoionization of these 4l4l' states into the n = 2 continuum. These experimental findings together with preliminary spectroscopic calculations concerning the configuration interaction of the Ne 8+ (4l4l') states with the Ne 8+ (3lnl') Rydberg series are also discussed within the context of the electron stabilization which follows a double capture. (Author)

Formation of cold molecules through the photo-association of cold atoms of Cesium. Existence of long range forces between between cold excited atoms of Cesium

International Nuclear Information System (INIS)

Comparat, D.

1999-09-01

This thesis deals with the experimental study and the theoretical interpretation of the processes involved in photo-association and the formation of cold caesium molecules. It also presents a study of the dipolar forces between a pair of cold excited caesium atoms. We present here the first photo-association experiment on cold caesium atoms: two cold atoms absorb a photon to form an excited electronically excited molecules in a rotation-vibration level. The first production of cold molecules which was realised experimentally, after the spontaneous deexcitation of the photo-associated molecules, is described, stressing the role of the potential well of the molecular states O g - (6s+6p 3/2 ) or 1 u (6s+6p 3/2 ) of caesium. The detection of the formed caesium molecules is based on a two-photons resonant ionisation that creates Cs 2 + ions, afterwards selectively detected. Temperatures around 20-200 μK have been measured. The photo-associative spectroscopy is described on the theoretical point of view: a detailed theoretical study allows to calculate precisely the asymptotic parts of the potential curves. On the experimental point of view, we present the spectroscopy of the extern potential well of the caesium state O g - (6s+6p 3/2 ) and the construction of an effective potential curve of the RKR type. A unified theory of photo-association in weak field, considered as a collision assisted by laser, is developed. The cold atoms experiments allow to study and control the collision between two atoms whose mutual interaction is of the dipole-dipole type. Two different physical systems are studied: a sample of Rydberg atoms, and the photo-association process which is a laser-assisted collision. A modification of the motion of one pair of atoms makes it possible to control the bipolar forces and to choose the atoms relative speeds. (author)

Predissociation of high-lying Rydberg states of molecular iodine via ion-pair states

Energy Technology Data Exchange (ETDEWEB)

Bogomolov, Alexandr S. [Institute of Chemical Kinetics and Combustion, Institutskaya Str. 3, Novosibirsk 630090 (Russian Federation); Grüner, Barbara; Mudrich, Marcel [Physikalisches Institut, Universität Freiburg, D-79104 Freiburg (Germany); Kochubei, Sergei A. [Institute of Semiconductor Physics, ac. Lavrent' yev ave., 13, Novosibirsk 630090 (Russian Federation); Baklanov, Alexey V. [Institute of Chemical Kinetics and Combustion, Institutskaya Str. 3, Novosibirsk 630090 (Russian Federation); Novosibirsk State University, Pirogova Str. 2, Novosibirsk 630090 (Russian Federation)

2014-03-28

Velocity map imaging of the photofragments arising from two-photon photoexcitation of molecular iodine in the energy range 73 500–74 500 cm{sup −1} covering the bands of high-lying gerade Rydberg states [{sup 2}Π{sub 1/2}]{sub c}6d;0{sub g}{sup +} and [{sup 2}Π{sub 1/2}]{sub c}6d;2{sub g} has been applied. The ion signal was dominated by the atomic fragment ion I{sup +}. Up to 5 dissociation channels yielding I{sup +} ions with different kinetic energies were observed when the I{sub 2} molecule was excited within discrete peaks of Rydberg states and their satellites in this region. One of these channels gives rise to images of I{sup +} and I{sup −} ions with equal kinetic energy indicating predissociation of I{sub 2} via ion-pair states. The contribution of this channel was up to about 50% of the total I{sup +} signal. The four other channels correspond to predissociation via lower lying Rydberg states giving rise to excited iodine atoms providing I{sup +} ions by subsequent one-photon ionization by the same laser pulse. The ratio of these channels varied from peak to peak in the spectrum but their total ionic signal was always much higher than the signal of (2 + 1) resonance enhanced multi-photon ionization of I{sub 2}, which was previously considered to be the origin of ionic signal in this spectral range. The first-tier E0{sub g}{sup +} and D{sup ′}2{sub g} ion-pair states are concluded to be responsible for predissociation of Rydberg states [{sup 2}Π{sub 1/2}]{sub c}6d;0{sub g}{sup +} and [{sup 2}Π{sub 1/2}]{sub c}6d;2{sub g}, respectively. Further predissociation of these ion-pair states via lower lying Rydberg states gives rise to excited I(5s{sup 2}5p{sup 4}6s{sup 1}) atoms responsible for major part of ion signal. The isotropic angular distribution of the photofragment recoil directions observed for all channels indicates that the studied Rydberg states are long-lived compared with the rotational period of the I{sub 2} molecule.

Calculation of Rydberg interaction potentials

DEFF Research Database (Denmark)

Weber, Sebastian; Tresp, Christoph; Menke, Henri

2017-01-01

for calculating the required electric multipole moments and the inclusion of electromagnetic fields with arbitrary direction. We focus specifically on symmetry arguments and selection rules, which greatly reduce the size of the Hamiltonian matrix, enabling the direct diagonalization of the Hamiltonian up...... to higher multipole orders on a desktop computer. Finally, we present example calculations showing the relevance of the full interaction calculation to current experiments. Our software for calculating Rydberg potentials including all features discussed in this tutorial is available as open source....

Auto transfer to Rydberg states and indirect stabilization following double capture

Energy Technology Data Exchange (ETDEWEB)

Roncin, P.; Gaboriaud, M.N.; Barat, M. (Paris-11 Univ., 91 - Orsay (France)); Bordenave-Montesquieu, A.; Moretto-Capelle, P.; Benhenni, M. (Toulouse-3 Univ., 31 (France)); Bachau, H.; Harel, C. (Bordeaux-1 Univ., 33 (France))

1993-11-28

Two-electron capture by slow multiply charged ions colliding on rare-gas target at keV energies is known to populate doubly excited states of the projectile with large cross sections. Though these states are dominantly autoionizing, important radiative decay following double capture have been reported, among which the direct observation of the fluorescence from Rydberg states. A mechanism based on post-collisional effects was proposed, in which Rydberg states are fed from the quasi-symmetrical doubly excited states initially populated. In this paper, a quantitative analysis of this effect is developed leading to a simple model which is applied to N[sup 7+] on He and Ar collisions. (author).

Auto transfer to Rydberg states and indirect stabilization following double capture

International Nuclear Information System (INIS)

Roncin, P.; Gaboriaud, M.N.; Barat, M.; Bordenave-Montesquieu, A.; Moretto-Capelle, P.; Benhenni, M.; Bachau, H.; Harel, C.

1993-01-01

Two-electron capture by slow multiply charged ions colliding on rare-gas target at keV energies is known to populate doubly excited states of the projectile with large cross sections. Though these states are dominantly autoionizing, important radiative decay following double capture have been reported, among which the direct observation of the fluorescence from Rydberg states. A mechanism based on post-collisional effects was proposed, in which Rydberg states are fed from the quasi-symmetrical doubly excited states initially populated. In this paper, a quantitative analysis of this effect is developed leading to a simple model which is applied to N 7+ on He and Ar collisions. (author)

Systematics in Rydberg state excitations for ion-atom collisions

International Nuclear Information System (INIS)

Andresen, B.; Jensen, K.; Petersen, N.B.; Veje, E.

1976-01-01

Rydberg state excitations in the Ne + , Mg + -He collisions have been studied in the projectile energy range 10-75 keV by means of optical spectrometry in a search for systematic trends. The relative excitation cross sections for levels of a Rydberg term series are found to follow a general (nsup(x))sup(P) behaviour with P < approximately -3 varying with collision energy and particles, regardless of whether the excited state population results from direct excitation, single electron transfer, or double electron transfer. At higher collision energies P is approximately -3 as predicted by theory. Polarization of the emitted line radiation indicates that there is no general rule for the relative excitation of the different magnetic substates of the same level. A statistical distribution of excitation is found for levels within the same term when the fine structure splitting is small. (Auth.)

Mean-field energy-level shifts and dielectric properties of strongly polarized Rydberg gases

OpenAIRE

Zhelyazkova, V.; Jirschik, R.; Hogan, S. D.

2016-01-01

Mean-field energy-level shifts arising as a result of strong electrostatic dipole interactions within dilute gases of polarized helium Rydberg atoms have been probed by microwave spectroscopy. The Rydberg states studied had principal quantum numbers n=70 and 72, and electric dipole moments of up to 14 050 D, and were prepared in pulsed supersonic beams at particle number densities on the order of 108 cm−3. Comparisons of the experimental data with the results of Monte Carlo calculations highl...

Cold atoms in a cryogenic environment

International Nuclear Information System (INIS)

Haslinger, S.

2011-01-01

The idea of quantum information processing attracts increasingly interest, where a complex collection of quantum objects and quantum bits are employed to find the ideal building blocks for quantum information systems. Hybrid quantum systems are therefore promising objects as they countervail the particular drawbacks of single quantum objects. Based on superconducting resonator technology, microwave coplanar waveguides provide a well suited interconnection for photons and solid-state quantum bits (qubits), extensively investigated in recent years. Since a quantum memory is presently missing in those electrical accessible circuit cavity quantum devices, connecting the fast processing in a solid sate device to the exceptional long coherence times in atomic ensembles, the presented work is focused to establish the technological foundations for the hybridization of such quantum systems. The microwave photons stored in a superconducting high finesse microwave resonator are therefore an ideal connection between the atom and the solid state quantum world. In the last decade, the miniaturization and integration of quantum optics and atomic physics manipulation techniques on to a single chip was successfully established. Such atom chips are capable of detailed quantum manipulation of ultra-cold atoms and provide a versatile platform to combine the manipulation techniques from atomic physics with the capability of nano-fabrication. In recent years several experiments succeeded in realization of superconducting atom chips in cryogenic environments which opens the road for integrating super-conductive microwave resonators to magnetically couple an atomic ensemble to photons stored in the coplanar high finesse cavity. This thesis presents the concept, design and experimental setup of two approaches to establish an atomic ensemble of rubidium atoms inside a cryogenic environment, based on an Electron beam driven alkali metal atom source for loading a magneto optical trap in a

Vanadium, rubidium and potassium in Octopus vulgaris (Mollusca: Cephalopoda

Directory of Open Access Journals (Sweden)

Sónia Seixas

2005-06-01

Full Text Available The levels of vanadium, rubidium and potassium were determined in Octopus vulgaris caught during commercial fishing activities at three locations (Cascais, Santa Luzia and Viana do Castelo in Portugal in autumn and spring. We determined the concentration of these elements in digestive gland, branchial heart, gills, mantle and arms in males and females. At least five males and five females were assessed for each season/location combination. Elemental concentrations were determined by Particle Induced X-ray Emission (PIXE. Vanadium was detectable only in digestive gland and branchial heart samples. Its concentration was not correlated with total weight, total length or mantle length. There were no differences in concentrations of V, Rb and K between sexes. There were significant differences in vanadium concentrations in branchial hearts in autumn between samples from Viana do Castelo and those from the other two sites. We found a significant positive relationship between the concentration of vanadium and those of potassium and rubidium in branchial hearts. Branchial hearts appear to play an important role in decontamination of V.

MgH Rydberg series: Transition energies from electron propagator theory and oscillator strengths from the molecular quantum defect orbital method

Science.gov (United States)

Corzo, H. H.; Velasco, A. M.; Lavín, C.; Ortiz, J. V.

2018-02-01

Vertical excitation energies belonging to several Rydberg series of MgH have been inferred from 3+ electron-propagator calculations of the electron affinities of MgH+ and are in close agreement with experiment. Many electronically excited states with n > 3 are reported for the first time and new insight is given on the assignment of several Rydberg series. Valence and Rydberg excited states of MgH are distinguished respectively by high and low pole strengths corresponding to Dyson orbitals of electron attachment to the cation. By applying the Molecular Quantum Defect Orbital method, oscillator strengths for electronic transitions involving Rydberg states also have been determined.

Optical coupling of cold atoms to a levitated nanosphere

Science.gov (United States)

Montoya, Cris; Witherspoon, Apryl; Fausett, Jacob; Lim, Jason; Kitching, John; Geraci, Andrew

2017-04-01

Cooling mechanical oscillators to their quantum ground state enables the study of quantum phenomena at macroscopic levels. In many cases, the temperature required to cool a mechanical mode to the ground state is below what current cryogenic systems can achieve. As an alternative to cooling via cryogenic systems, it has been shown theoretically that optically trapped nanospheres could reach the ground state by sympathetically cooling the spheres via cold atoms. Such cooled spheres can be used in quantum limited sensing and matter-wave interferometry, and could also enable new hybrid quantum systems where mechanical oscillators act as transducers. In our setup, optical fields are used to couple a sample of cold Rubidium atoms to a nanosphere. The sphere is optically levitated in a separate vacuum chamber, while the atoms are trapped in a 1-D optical lattice and cooled using optical molasses. This work is partially supported by NSF, Grant No. PHY-1506431.

Lithium atoms on helium nanodroplets: Rydberg series and ionization dynamics

Science.gov (United States)

Lackner, Florian; Krois, Günter; Ernst, Wolfgang E.

2017-11-01

The electronic excitation spectrum of lithium atoms residing on the surface of helium nanodroplets is presented and analyzed employing a Rydberg-Ritz approach. Utilizing resonant two-photon ionization spectroscopy, two different Rydberg series have been identified: one assigned to the nS(Σ) series and the other with predominantly nP(Π) character. For high Rydberg states, which have been resolved up to n = 13, the surrounding helium effectively screens the valence electron from the Li ion core, as indicated by the apparent red-shift of Li transitions and lowered quantum defects on the droplet with respect to their free atom counterparts. For low n states, the screening effect is weakened and the prevailing repulsive interaction gives rise to strongly broadened and blue-shifted transitions. The red-shifts originate from the polarization of nearby He atoms by the positive Li ion core. As a consequence of this effect, the ionization threshold is lowered by 116 ± 10 cm-1 for Li on helium droplets with a radius of about 40 Å. Upon single-photon ionization, heavy complexes corresponding to Li ions attached to intact helium droplets are detected. We conclude that ionization close to the on-droplet ionization threshold triggers a dynamic process in which the Li ion core undergoes a transition from a surface site into the droplet.

Sympathetic cooling of ytterbium with rubidium; Sympathetische Kuehlung von Ytterbium mit Rubidium

Energy Technology Data Exchange (ETDEWEB)

Tassy, S.

2007-12-14

Within the scope of this thesis, a mixture of ultracold ytterbium and rubidium atoms was experimentally realized and investigated. For these experiments, a novel trap geometry was developed which allows simultaneous trapping and cooling of diamagnetic and paramagnetic atomic species. The main focus was put on the investigation of the interspecies scattering properties, where sympathetic cooling of ytterbium through elastic collisions with rubidium could be demonstrated. In addition, the interspecies scattering length could be determined. In the current configuration the combined trap allows the preparation of up to 2.10{sup 5} atoms of {sup 170}Yb, {sup 171}Yb, {sup 172}Yb, {sup 174}Yb or {sup 176}Yb at a temperature of 40..60 {mu}K and a density in the range of 10{sup 12} cm{sup -3}, and of about 10{sup 7} {sup 87}Rb atoms at a temperature of 25 {mu}K and a density in the range of 5.10{sup 11} cm{sup -3}. Detailed studies of the thermalization of bosonic {sup 170}Yb, {sup 172}Yb, {sup 174}Yb and {sup 176}Yb and of fermionic {sup 171}Yb each with {sup 87}Rb were performed under varying experimental conditions. The deduced total scattering cross section was clearly found to increase with higher mass of the ytterbium isotope. In general, a mass scaling of the scattering properties is in agreement with theoretical models and former experimental work. With the assumption of pure s-wave scattering, which is approximately fulfilled for the given experimental parameters, the interspecies scattering length could be derived from the measured thermalization data and was found to be (in units of the Bohr radius a{sub 0}): {sup 170}Yb-{sup 87}Rb:(18{sup +12}{sub -4})a{sub 0}, {sup 171}Yb-{sup 87}Rb:(25{sup +14}{sub -7})a{sub 0}, {sup 172}Yb-{sup 87}Rb:(33{sup +23}{sub -7})a{sub 0}, {sup 174}Yb-{sup 87}Rb:(83{sup +89}{sub -25})a{sub 0}, {sup 176}Yb-{sup 87}Rb:(127{sup +245}{sub -45})a{sub 0}. (orig./HSI)

Rubidium dimers in paraffin-coated cells

International Nuclear Information System (INIS)

Acosta, V M; Windes, D; Corsini, E; Ledbetter, M P; Karaulanov, T; Budker, D; Jarmola, A; Auzinsh, M; Rangwala, S A; Jackson Kimball, D F

2010-01-01

Measurements were made to determine the density of rubidium dimer vapor in paraffin-coated cells. The number density of dimers and atoms in similar paraffin-coated and uncoated cells was measured by optical spectroscopy. Due to the relatively low melting point of paraffin, a limited temperature range of 43-80 0 C was explored, with the lower end corresponding to a dimer density of less than 10 7 cm -3 . With 1 min integration time, a sensitivity to dimer number density of better than 10 6 cm -3 was achieved. No significant difference in dimer density between the cells was observed.

Alkali Rydberg states in electromagnetic fields: computational physics meets experiment

International Nuclear Information System (INIS)

Krug, A.

2001-11-01

We study highly excited hydrogen and alkali atoms ('Rydberg states') under the influence of a strong microwave field. As the external frequency is comparable to the highly excited electron's classical Kepler frequency, the external field induces a strong coupling of many different quantum mechanical energy levels and finally leads to the ionization of the outer electron. While periodically driven atomic hydrogen can be seen as a paradigm of quantum chaotic motion in an open (decaying) quantum system, the presence of the non-hydrogenic atomic core - which unavoidably has to be treated quantum mechanically - entails some complications. Indeed, laboratory experiments show clear differences in the ionization dynamics of microwave driven hydrogen and non-hydrogenic Rydberg states. In the first part of this thesis, a machinery is developed that allows for numerical experiments on alkali and hydrogen atoms under precisely identical laboratory conditions. Due to the high density of states in the parameter regime typically explored in laboratory experiments, such simulations are only possible with the most advanced parallel computing facilities, in combination with an efficient parallel implementation of the numerical approach. The second part of the thesis is devoted to the results of the numerical experiment. We identify and describe significant differences and surprising similarities in the ionization dynamics of atomic hydrogen as compared to alkali atoms, and give account of the relevant frequency scales that distinguish hydrogenic from non-hydrogenic ionization behavior. Our results necessitate a reinterpretation of the experimental results so far available, and solve the puzzle of a distinct ionization behavior of periodically driven hydrogen and non-hydrogenic Rydberg atoms - an unresolved question for about one decade. Finally, microwave-driven Rydberg states will be considered as prototypes of open, complex quantum systems that exhibit a complicated temporal decay

Electric Dipole Echoes in Rydberg Atoms

International Nuclear Information System (INIS)

Yoshida, S.; Reinhold, C. O.; Burgdoerfer, J.; Zhao, W.; Mestayer, J. J.; Lancaster, J. C.; Dunning, F. B.

2007-01-01

We report the first observation of echoes in the electric dipole moment of an ensemble of Rydberg atoms precessing in an external electric field F. Rapid reversal of the field direction is shown to play a role similar to that of a π pulse in NMR in rephasing a dephased ensemble of electric dipoles resulting in the buildup of an echo. The mechanisms responsible for this are discussed with the aid of classical trajectory Monte Carlo simulations

Concentration differences between serum and plasma of the elements cobalt, iron, mercury, rubidium, selenium and zinc determined by neutron activation analysis

International Nuclear Information System (INIS)

Kasperek, K.; Kiem, J.; Iyengar, G.V.; Feinendegen, L.E.

1981-01-01

The differences in concentrations of cesium, cobalt, iron, mercury, rubidium, selenium and zinc between serum and plasma were examined with the aid of instrumental neutron activation analysis. Eighty serum and plasma samples obtained from 13 donors were compared. Serum was prepared in plastic tubes immediately after clotting, and plasma was separated with heparin as anticoagulant. No significant differences in the concentrations of cesium, cobalt, mercury and selenium were observed. However, the concentrations of iron, rubidium and zinc were significantly higher in serum than in plasma. The average differences were 322, 12 and 20 ng/ml for iron, rubidium and zinc, respectively. The average differences found for cesium, rubidium and zinc were far below that which can be expected from a complete, or considerable release of these elements from platelets which aggregate or disintegrate during the clotting process in preparing serum. (orig.)

Investigation by high resolution electron spectroscopy of the helium-like 3lnl' Rydberg series in double capture processes at low collision velocity: auto transfer to Rydberg states and electron stabilization

Energy Technology Data Exchange (ETDEWEB)

Bordenave-Montesquieu, A.; Moretto-Capelle, P.; Gonzalez, A.; Benhenni, M. (Toulouse-3 Univ., 31 (France)); Bachau, H.; Sanchez, I. (Bordeaux-1 Univ., 33 - Talence (France). Lab. des Collisions Atomiques)

1994-09-28

A high resolution electron spectrometry of the (3lnl') Ryberg series populated in N[sup 7+] + He and Ne[sup 10+] + He collisions at 10 q keV, 10[sup o] allows us to observe, for the first time by this method, two post-collisional effects. First, it is found with nitrogen ions that, when n increases from n = 4 to 9, the L-distribution peaks more and more on the high angular momentum states. This is qualitatively understood as a Stark deformation of the Rydberg orbit by the Coulomb field of the receding ion. Also, in the n range where the double capture process populates symmetrical 4l4l' states (n>9), an enhancement of the intensities of the 3lnl' Rydberg lines is observed for both collisonal systems. This is thought to be a signature of the so-called auto transfer to Rydberg states effect. The transfer of population from the 3l4l' to the 3lnl' states is found to be favoured against a direct autoionization of these 4l4l' states into the n = 2 continuum. These experimental findings together with preliminary spectroscopic calculations concerning the configuration interaction of the Ne[sup 8+] (4l4l') states with the Ne[sup 8+](3lnl') Rydberg series are also discussed within the context of the electron stabilization which follows a double capture. (Author).

Analytical investigation of one-dimensional Rydberg atoms interacting with half-cycle pulses

International Nuclear Information System (INIS)

Bersons, I.; Veilande, R.

2004-01-01

Classical, quantum-mechanical, and semiclassical expressions for the transition probability in one-dimensional Rydberg atom irradiated by short half-cycle pulse are derived and compared. The simple formulas obtained for excitation of Rydberg atom by two time delayed weak half-cycle pulses reproduce well the experimental data and the solutions of time-dependent Schroedinger equation. When the transferred momenta are stronger and positive, the transition probabilities exhibit fast oscillations with time delay between the pulses. The classical transition probability is constant in time. For negative transferred momenta a focusing phenomenon is observed, and there is a region in time delay, where the transition probabilities oscillate with the Kepler period

Hydrogen Balmer series measurements and determination of Rydberg's constant using two different spectrometers

International Nuclear Information System (INIS)

Amrani, D

2014-01-01

This paper investigates the use of two different methods, the optical and the computer-aided diffraction-grating spectrometer, to measure the wavelength of visible lines of Balmer series from the hydrogen atomic spectrum and estimate the value of Rydberg's constant. Analysis and interpretation of data showed that both methods, despite their difference in terms of the type of equipment used, displayed good performance in terms of precision of measurements of wavelengths of spectral lines. A comparison was carried out between the experimental value of Rydberg's constant obtained with both methods and the accepted value. The results of Rydberg's constant obtained with both the optical and computer-aided spectrometers were 1.099 28 × 10 −7  m −1  and 1.095 13 × 10 −7  m −1  with an error difference of 0.17% and 0.20% compared to the accepted value 1.097 373 × 10 −7  m −1 , respectively. (paper)

Creating high-purity angular-momentum-state Rydberg atoms by a pair of unipolar laser pulses

Science.gov (United States)

Xin, PeiPei; Cheng, Hong; Zhang, ShanShan; Wang, HanMu; Xu, ZiShan; Liu, HongPing

2018-04-01

We propose a method of producing high-purity angular-momentum-state Rydberg atoms by a pair of unipolar laser pulses. The first positive-polarity optical half-cycle pulse is used to prepare an excited-state wave packet while the second one is less intense, but with opposite polarity and time delayed, and is employed to drag back the escaping free electron and clip the shape of the bound Rydberg wave packet, selectively increasing or decreasing a fraction of the angular-momentum components. An intelligent choice of laser parameters such as phase and amplitude helps us to control the orbital-angular-momentum composition of an electron wave packet with more facility; thus, a specified angular-momentum state with high purity can be achieved. This scheme of producing high-purity angular-momentum-state Rydberg atoms has significant application in quantum-information processing.

Auto transfer to Rydberg states during ion-atom collisions

International Nuclear Information System (INIS)

Bachau, H.; Harel, C.; Barat, M.; Roncin, P.; Bordenave-Montesquieu, A.; Moretto-Capelle, P.; Benoit-Cattin, P.; Gleizes, A.; Benhenni, M.

1993-01-01

Electron capture by slow multiply charged ions colliding on rare-gas targets is known to populate highly excited states of the projectile. On the basis of experimental measurement of energy and angle differential cross-sections we have shown that capture to a resonant doubly excited state may lead to Autoionizing Double Capture (ADC) as well as to True Double Capture (TDC). In this model TDC appears as a two step post-collisional process, the state populated by the collision decays to (or delutes into) a dense adjacent Rydberg series, followed by radiative deexcitation of the inner electron of the (3,n) Rydberg states. We report here new experimental observations in electron spectra measured in N 7+ +He. Auto transfer to Rydber states has also important consequences on the determination of the lifetime of the autoionizing states, some discrepancies between theoretical width values for low N 5+ (4,4) resonant states will be discussed and partially resolved

Auto transfer to Rydberg states during ion-atom collisions

Energy Technology Data Exchange (ETDEWEB)

Bachau, H.; Harel, C. (Laboratoire des Collisions Atomiques, Unite Propre de Recherche 260 du CNRS, Universite Bordeaux I, 351 Cours de la Liberation, 33405 Talence (France)); Barat, M.; Roncin, P. (Laboratoire des Collisions Atomiques et Moleculaires, Unite associee 281 du CNRS, Universite de Paris Sud, Batiment 351, 91405 Orsay (France)); Bordenave-Montesquieu, A.; Moretto-Capelle, P.; Benoit-Cattin, P.; Gleizes, A.; Benhenni, M. (IRSAMC, Unite associee 770 du CNRS, Universite Paul Sabatier, 118 route de Narbonne, 31062 Toulouse (France))

1993-06-05

Electron capture by slow multiply charged ions colliding on rare-gas targets is known to populate highly excited states of the projectile. On the basis of experimental measurement of energy and angle differential cross-sections we have shown that capture to a resonant doubly excited state may lead to Autoionizing Double Capture (ADC) as well as to True Double Capture (TDC). In this model TDC appears as a two step post-collisional process, the state populated by the collision decays to (or delutes into) a dense adjacent Rydberg series, followed by radiative deexcitation of the inner electron of the (3,n) Rydberg states. We report here new experimental observations in electron spectra measured in [ital N][sup 7+]+[ital He]. Auto transfer to Rydber states has also important consequences on the determination of the lifetime of the autoionizing states, some discrepancies between theoretical width values for low [ital N][sup 5+](4,4) resonant states will be discussed and partially resolved.

From the Rydberg constant to the fundamental constants metrology

International Nuclear Information System (INIS)

Nez, F.

2005-06-01

This document reviews the theoretical and experimental achievements of the author since the beginning of his scientific career. This document is dedicated to the spectroscopy of hydrogen, deuterium and helium atoms. The first part is divided into 6 sub-sections: 1) the principles of hydrogen spectroscopy, 2) the measurement of the 2S-nS/nD transitions, 3) other optical frequency measurements, 4) our contribution to the determination of the Rydberg constant, 5) our current experiment on the 1S-3S transition, 6) the spectroscopy of the muonic hydrogen. Our experiments have improved the accuracy of the Rydberg Constant by a factor 25 in 15 years and we have achieved the first absolute optical frequency measurement of a transition in hydrogen. The second part is dedicated to the measurement of the fine structure constant and the last part deals with helium spectroscopy and the search for optical references in the near infrared range. (A.C.)

The l-mixing cross section of Rydberg states of atomic Rb and the scaling LAW

International Nuclear Information System (INIS)

Liu Hong; Chen Aiqiu; Li Baiwen

1991-01-01

On the basis of impulse approximate method, a kind of analytical wavefunctions based on a potential model was used to calculate the l mixing cross section of thermal collision of Rydberg states of atomic Rb with rare gas (He, Ne). The results were compared with the experimental results and other theoretical values. These results show that there exists a kind of scaling law for the l mixing cross section of Rydberg alkali atoms

Cavity quantum electrodynamics with a Rydberg-blocked atomic ensemble

DEFF Research Database (Denmark)

Guerlin, Christine; Brion, Etienne; Esslinger, Tilman

2010-01-01

The realization of a Jaynes-Cummings model in the optical domain is proposed for an atomic ensemble. The scheme exploits the collective coupling of the atoms to a quantized cavity mode and the nonlinearity introduced by coupling to high-lying Rydberg states. A two-photon transition resonantly cou...

Survival of Rydberg atoms in intense laser fields and the role of nondipole effects

Science.gov (United States)

Klaiber, Michael; Dimitrovski, Darko

2015-02-01

We consider the interaction of Rydberg atoms with strong infrared laser pulses using an approach based on the Magnus expansion of the time evolution operator. First-order corrections beyond the electric dipole approximation are also included in the theory. We illustrate the dynamics of the interaction at the parameters of the experiment [Eichmann et al., Phys. Rev. Lett. 110, 203002 (2013), 10.1103/PhysRevLett.110.203002]. It emerges that the depletion of Rydberg atoms in this regime comes predominantly from the nondipole effects.

Observations of cold antihydrogen

CERN Document Server

Tan, J N; Gabrielse, G; Oxley, P; Speck, A; Storry, C H; Wessels, M; Grzonka, D; Oelert, W; Schepers, G; Sefzick, T; Walz, J; Pittner, H; Hänsch, T W; Hessels, E A

2004-01-01

ATRAP's e/sup +/ cooling of p in a nested Penning trap has led to reports of cold H produced during such cooling by the ATHENA and ATRAP collaborations. To observe H, ATHENA uses coincident annihilation detection and ATRAP uses field ionization followed by p storage. Advantages of ATRAP's field ionization method include the complete absence of any background events, and the first way to measure which H states are produced. ATRAP enhances the H production rate by driving many cycles of e/sup +/ cooling in the nested trap, with more H counted in an hour than the sum of all the other antimatter atoms ever reported. The number of H counted per incident high energy p is also higher than ever observed. The first measured distribution of H states is made using a pre-ionizing electric field between separated production and detection regions. The high rate and the high Rydberg states suggest that the H is formed via three-body recombination, as expected. (22 refs).

Rydberg states of chloroform studied by VUV photoabsorption spectroscopy

Science.gov (United States)

Singh, Param Jeet; Shastri, Aparna; D'Souza, R.; Jagatap, B. N.

2013-11-01

The VUV photoabsorption spectra of CHCl3 and CDCl3 in the energy region 6.2-11.8 eV (50,000-95,000 cm-1) have been investigated using synchrotron radiation from the Indus-1 source. Rydberg series converging to the first four ionization limits at 11.48, 11.91, 12.01 and 12.85 eV corresponding to excitation from the 1a2, 4a1, 4e, 3e, orbitals of CHCl3 respectively are identified and analyzed. Quantum defect values are observed to be consistent with excitation from the chlorine lone pair orbitals. Vibrational progressions observed in the region of 72,500-76,500 cm-1 have been reassigned to ν3 and combination modes of ν3+ν6 belonging to the 1a2→4p transition in contrast to earlier studies where they were assigned to a ν3 progression superimposed on the 3e→4p Rydberg transition. The assignments are further confirmed based on isotopic substitution studies on CDCl3 whose VUV photoabsorption spectrum is reported here for the first time. The frequencies of the ν3 and ν6 modes in the 4p Rydberg state of CHCl3 (CDCl3) are proposed to be ~454 (409) cm-1 and~130 (129) cm-1 respectively based on the vibronic analysis. DFT calculations of neutral and ionic ground state vibrational frequencies support the vibronic analysis. Experimental spectrum is found to be in good agreement with that predicted by TDDFT calculations. This work presents a consolidated analysis of the VUV photoabsorption spectrum of chloroform.

New innershell phenomena from Rydberg series of highly charged ions

International Nuclear Information System (INIS)

Rosmej, F.B.

1997-01-01

Dielectronic satellite spectra near the He-like resonance line W are investigated experimentally and theoretically. We propose that under certain plasma conditions the resonance line structure plays a minor role and can be mixed with the accumulation of Rydberg satellites. (orig.)

Topological matter with collective encoding and Rydberg blockade

DEFF Research Database (Denmark)

Nielsen, Anne E. B.; Mølmer, Klaus

2010-01-01

We propose to use a permutation symmetric sample of multilevel atoms to simulate the properties of topologically ordered states. The Rydberg blockade interaction is used to prepare states of the sample which are equivalent to resonating valence bond states, Laughlin states, and string-net condens......-net condensates and to create and study the properties of their quasi-particle-like fundamental excitations....

Population of Rydberg states by electron capture in fast-ion--atom collisions

International Nuclear Information System (INIS)

Burgdoerfer, J.; Dube, L.J.

1985-01-01

The l,m-substate distribution in low-lying Rydberg manifolds (nroughly-equal10) following electron capture H + +H(1s)→H(n)+H + is calculated at high velocities (v>1 a.u.) in the continuum-distorted-wave (CDW) approximation. The standard CDW approximation is modified to account for final-state Stark mixing of the Rydberg manifold in the exit channel using the post-collision-interaction model. The influence of multiple-scattering contributions is analyzed and comparison is made with sigma/sub l/m predicted by the Born approximation. We find that the double-scattering contribution, closely connected with the classical Thomas process, becomes visible in the CDW approximation at surprisingly low nonasymptotic velocities

Laser diagnostics of the energy spectrum of Rydberg states of the lithium-7 atom

Energy Technology Data Exchange (ETDEWEB)

Zelener, B. B., E-mail: bobozel@mail.ru; Saakyan, S. A.; Sautenkov, V. A.; Manykin, E. A.; Zelener, B. V.; Fortov, V. E. [Russian Academy of Sciences, Joint Institute for High Temperatures (Russian Federation)

2015-12-15

The spectra of excited lithium-7 atoms prepared in a magneto-optical trap are studied using a UV laser. The laser diagnostics of the energy of Rydberg atoms is developed based on measurements of the change in resonance fluorescence intensity of ultracold atoms as the exciting UV radiation frequency passes through the Rydberg transition frequency. The energies of various nS configurations are obtained in a broad range of the principal quantum number n from 38 to 165. The values of the quantum defect and ionization energy obtained in experiments and predicted theoretically are discussed.

Early risk stratification using Rubidium-82 positron emission tomography in STEMI patients

DEFF Research Database (Denmark)

Ghotbi, Adam Ali; Hasbak, Philip; Nepper-Christensen, Lars

2018-01-01

BACKGROUND: Assessment of infarct size after myocardial infarction is predictive of subsequent morphological changes and clinical outcome. This study aimed to assess subacute post-intervention Rubidium-82 ((82)Rb)-PET imaging in predicting left ventricle ejection fraction, regional wall motion, a...

New innershell phenomena from Rydberg series of highly charged ions

Energy Technology Data Exchange (ETDEWEB)

Rosmej, F.B. [Bochum Univ. (Germany). Inst. fuer Experimentalphysik; Faenov, A.Ya. [MISDC, VNIIFTRI, Mendeleevo (Russian Federation)

1997-12-31

Dielectronic satellite spectra near the He-like resonance line W are investigated experimentally and theoretically. We propose that under certain plasma conditions the resonance line structure plays a minor role and can be mixed with the accumulation of Rydberg satellites. (orig.). 7 refs.

Realization of a frequency standard at 778 nm: absolute frequency measurement of the 2S-8S/D transitions in hydrogen and deuterium and determination of the Rydberg constant; Realisation d'un etalon de frequence a 778 nm: mesure absolue des frequences 2S-8S/D des atomes d'hydrogene et de deuterium et determination de la constante de rydberg

Energy Technology Data Exchange (ETDEWEB)

Beauvoir, B. de

1996-12-15

The purpose of this work is to design a 778 nm standard laser for performing an absolute measurement of 2S-8S/D frequencies of hydrogen and deuterium atoms. This frequency calibration is based on a 5S-5D two-photon transition of the rubidium atom. Metrological performance of this laser is 10 times as good as that of He-Ne laser calibrated on iodine. It has been shown that the passage of a laser radiation through an optic fiber does not deteriorate its metrological properties. 2S-8S/8D transitions have been excited in an atomic jet by a titanium-sapphire laser. Spurious effects can shift and broaden lines. In order to prevent these effects, a theoretical line has been shaped and adjusted on experimental signals. The frequency comparison between the excitation laser and the standard laser has led to the measurement of the absolute frequency of the line concerned. The value of the Rydberg constant has been deduced: R{sub {infinity}} = 109737.3156859 (10) cm{sup -1}. The comparison of experimental data between deuterium and hydrogen has allowed us to determine the value of the Lamb shift of the 2S state of deuterium: L(2S-2P) = 1059,230 (9) MHz.

The Closed-Orbit Theory for General Rydberg Atoms in External Fields

International Nuclear Information System (INIS)

Carboni, R.

1997-01-01

The photoabsorption spectra of hydrogen Rydberg atoms, as well of model Rydberg atoms in pure magnetic or electric fields have been successfully calculated using the semiclassical closed-orbit theory. The theory relates the resonances of the spectra to closed classical orbits of the excited electron. The dynamics of multielectron atoms is more complicated than the hydrogenic one; additionally, when the atoms are in the presence of perpendicular magnetic and electric fields becomes more complex than when they are in pure fields, due to the fact that the Hamiltonian is non-separable in three degrees of freedom, instead of two non-separable degrees of freedom. In this work, I present an extension of the closed-orbit theory to three degrees of freedom, considering arbitrary quantum defects, i.e., general atoms. (Author) [es

Positive-column plasma studied by fast-flow glow discharge mass spectrometry: Could it be a 'Rydberg gas?'

International Nuclear Information System (INIS)

Mason, Rod S.; Miller, Pat D.; Mortimer, Ifor; Mitchell, David J.; Dash, Neil A.

2003-01-01

Ions created from the fast-flowing positive column plasma of a glow discharge were monitored using a high voltage magnetic sector mass spectrometer. Since the field gradient and sheath potentials created by the plasma inside the source opposed cation transfer, it is inferred that the ions detected were the field-ionized Rydberg species. This is supported by the mass spectral changes which occurred when a negative bias was applied to the sampling aperture and by the contrasting behavior when attached to a quadrupole analyzer. Reaction with H 2 (titrated into the flowing plasma) quenched not only the ionization of discharge gas Rydberg atoms but also the passage of electric current through the plasma, without significant changes to the field and sheath potentials. Few 'free' ions were present and the lifetimes of the Rydberg atoms detected were much longer than seen in lower pressure experiments, indicating additional stabilization in the plasma environment. The observations support the model of the flowing plasma, given previously [R. S. Mason, P. D. Miller, and I. P. Mortimer, Phys. Rev. E 55, 7462 (1997)] as mainly a neutral Rydberg atom gas, rather than a conventional ion-electron plasma

Ionization of nS, nP, and nD lithium, potassium, and cesium Rydberg atoms by blackbody radiation

Science.gov (United States)

Beterov, I. I.; Ryabtsev, I. I.; Tretyakov, D. B.; Bezuglov, N. N.; Ékers, A.

2008-07-01

The results of theoretical calculations of the blackbody ionization rates of lithium, potassium, and cesium atoms residing in Rydberg states are presented. The calculations are performed for nS, nP, and nD states in a wide range of principal quantum numbers, n = 8-65, for blackbody radiation temperatures T = 77, 300, and 600 K. The calculations are performed using the known quasi-classical formulas for the photoionization cross sections and for the radial matrix elements of transitions in the discrete spectrum. The effect of the blackbody-radiation-induced population redistribution between Rydberg states on the blackbody ionization rates measured under laboratory conditions is quantitatively analyzed. Simple analytical formulas that approximate the numerical results and that can be used to estimate the blackbody ionization rates of Rydberg atoms are presented. For the S series of lithium, the rate of population of high-lying Rydberg levels by blackbody radiation is found to anomalously behave as a function of n. This anomaly is similar to the occurrence of the Cooper minimum in the discrete spectrum.

The determination of cesium and rubidium in highly radioactive waste liquid

International Nuclear Information System (INIS)

Wei Songsheng

1991-01-01

Cesium and rubidium in high-level waste liquid were determined by atomic absorption spectrometry with the instrument modified for analyzing radioactive samples. The results show that the method is effective and safe. The error of the method is less than +- 3%, and it has been used in the production of cesium

Thermodynamic properties of molten mixtures of lithium, rubidium, cesium and beryllium chlorides

International Nuclear Information System (INIS)

Zarubitskij, O.G.; Podafa, B.P.; Dubovoj, P.G.

1982-01-01

e. m. f. in binary systems of beryllium chloride with rubidium and cesium chlorides were measured. Concentration dependences of thermodynamic functions (mixing entropy Gibbs free energy) of beryllium chloride in the systems as well as with the participation of lithium chloride were analysed

Dissipative preparation of steady Greenberger-Horne-Zeilinger states for Rydberg atoms with quantum Zeno dynamics

Science.gov (United States)

Shao, X. Q.; Wu, J. H.; Yi, X. X.; Long, Gui-Lu

2017-12-01

Inspired by a recent work [F. Reiter, D. Reeb, and A. S. Sørensen, Phys. Rev. Lett. 117, 040501 (2016), 10.1103/PhysRevLett.117.040501], we present a simplified proposal for dissipatively preparing a Greenberger-Horne-Zeilinger (GHZ) state of three Rydberg atoms in a cavity. The Z pumping is implemented under the action of the spontaneous emission of Λ -type atoms and the quantum Zeno dynamics induced by strong continuous coupling. In the meantime, a dissipative Rydberg pumping breaks up the stability of the state | GHZ+〉 in the process of Z pumping, making | GHZ-〉 the unique steady state of the system. Compared with the former scheme, the number of driving fields acting on atoms is greatly reduced and only a single-mode cavity is required. The numerical simulation of the full master equation reveals that a high fidelity ˜98 % can be obtained with the currently achievable parameters in the Rydberg-atom-cavity system.

Electronic structure of molecular Rydberg states of some small molecules and molecular ion

International Nuclear Information System (INIS)

Sun Biao; Li Jiaming

1993-01-01

Based on an independent-particle-approximation (i.e. the multiple scattering self-consistent-field theory), the electronic structures of Rydberg states of the small diatomic molecules H 2 , He 2 and the He 2 + molecular ion were studied. The principal quantum number of the first state of the Rydberg series is determined from a convention of the limit of the molecular electronic configuration. The dynamics of the excited molecules and molecular ion has been elucidated. The theoretical results are in fair agreement with the existing experimental measurements, thus they can serve as a reliable basis for future refined treatment such as the configuration interaction calculation

Study on the application of crown ether for neutron activation analysis of rubidium and rhenium in rock samples

International Nuclear Information System (INIS)

Wang Xiaolin; Fu Yibei; Liu Yinong; Xiong Zonghua; Hao Fanhua

1996-01-01

The extraction behaviour of rubidium and rhenium with 18-crown-6 (18C6) and benzo-15-crown-5 (B15C5) in nitrobenzene from picric acid or potassium hydroxide solution are studied and methods for separation and determination are developed. The molar ratio of 18C6 to Rb and B15C5 to Re in the extracted species is probably 2:1. Rubidium and rhenium in rock samples are satisfactorily determined by neutron activation method

An investigation of electronic states of some molecules and molecular cations using mass analyzed threshold ionization and photoinduced Rydberg ionization spectroscopy

Science.gov (United States)

Hofstein, Jason David

1999-11-01

Mass analyzed threshold ionization (MATI) experiments have enabled mapping of the n-dependent Rydberg state survival probability for a series of molecules. Utilizing vacuum and extreme ultraviolet (VUV/XUV) photons, one photon Rydberg manifold spectra of argon, hydrogen chloride, nitrogen, benzene, and oxygen were produced, and the prospects of photoinduced Rydberg ionization (PIRI) experiments examined. It was found that the widths of Rydberg manifolds for the molecules studied are quite different. Hydrogen chloride and nitrogen have the narrowest manifold width, followed by benzene, and then oxygen. These varying widths are most strongly correlated with the angular momentum (i.e., quantum defect) of the initially prepared Rydberg orbital. PIRI experiments required the use of a static cell, rather than a molecular jet assembly, for the more efficient production of higher amounts of VUV/XUV radiation, and hence more Rydberg signal needed to observe PIRI. Armed with the ability to produce tunable VUV/XUV radiation, and to determine the feasibility of a PIRI experiment, the MATI and fragment PIRI spectra of trans-1,3-butadiene (BD) were recorded. The MATI spectrum is vibrationally resolved and was analyzed with the help of ab initio calculations and other published results. The fragment PIRI spectrum of the Aproduction of C3H3+ dominates, but at higher photon energies, C2H4 + is also produced. The production of each fragment showed a definite PIRI wavelength dependence.

Role of ion-pair states in the predissociation dynamics of Rydberg states of molecular iodine.

Science.gov (United States)

von Vangerow, J; Bogomolov, A S; Dozmorov, N V; Schomas, D; Stienkemeier, F; Baklanov, A V; Mudrich, M

2016-07-28

Using femtosecond pump-probe ion imaging spectroscopy, we establish the key role of I(+) + I(-) ion-pair (IP) states in the predissociation dynamics of molecular iodine I2 excited to Rydberg states. Two-photon excitation of Rydberg states lying above the lowest IP state dissociation threshold (1st tier) is found to be followed by direct parallel transitions into IP states of the 1st tier asymptotically correlating to a pair of I ions in their lowest states I(+)((3)P2) + I(-)((1)S0), of the 2nd tier correlating to I(+)((3)P0) + I(-)((1)S0), and of the 3rd tier correlating to I(+)((1)D2) + I(-)((1)S0). Predissociation via the 1st tier proceeds presumably with a delay of 1.6-1.7 ps which is close to the vibrational period in the 3rd tier state (3rd tier-mediated process). The 2nd tier IP state is concluded to be the main precursor for predissociation via lower lying Rydberg states proceeding with a characteristic time of 7-8 ps and giving rise to Rydberg atoms I(5s(2)5p(4)6s(1)). The channel generating I((2)P3/2) + I((2)P1/2) atoms with total kinetic energy corresponding to one-photon excitation is found to proceed via a pump - dump mechanism with dramatic change of angular anisotropy of this channel as compared with earlier nanosecond experiments.

Quantum localization of the kicked rydberg atom

Science.gov (United States)

Yoshida; Reinhold; Burgdorfer

2000-03-20

We investigate the quantum localization of the one-dimensional Rydberg atom subject to a unidirectional periodic train of impulses. For high frequencies of the train the classical system becomes chaotic and leads to fast ionization. By contrast, the quantum system is found to be remarkably stable. We find this quantum localization to be directly related to the existence of "scars" of the unstable periodic orbits of the system. The localization length is given by the energy excursion along the periodic orbits.

Fourier transform infrared emission spectra of atomic rubidium: g- and h-states

Czech Academy of Sciences Publication Activity Database

Civiš, Svatopluk; Ferus, Martin; Kubelík, Petr; Chernov, Vladislav E.; Zanozina, Ekaterina M.

2012-01-01

Roč. 45, č. 17 (2012), s. 175002 ISSN 0953-4075 R&D Projects: GA AV ČR IAAX00100903 Institutional support: RVO:61388955 Keywords : Fourier transform infrared emission spectra * atomic rubidium * physical chemistry Subject RIV: CF - Physical ; Theoretical Chemistry Impact factor: 2.031, year: 2012

Analyses of absorption distribution of a rubidium cell side-pumped by a Laser-Diode-Array (LDA)

Science.gov (United States)

Yu, Hang; Han, Juhong; Rong, Kepeng; Wang, Shunyan; Cai, He; An, Guofei; Zhang, Wei; Yu, Qiang; Wu, Peng; Wang, Hongyuan; Wang, You

2018-01-01

A diode-pumped alkali laser (DPAL) has been regarded as one of the most potential candidates to achieve high power performances of next generation. In this paper, we investigate the physical properties of a rubidium cell side-pumped by a Laser-Diode-Array (LDA) in this study. As the saturated concentration of a gain medium inside a vapor cell is extremely sensitive to the temperature, the populations of every energy-level of the atomic alkali are strongly relying on the vapor temperature. Thus, the absorption characteristics of a DPAL are mainly dominated by the temperature distribution. In this paper, the temperature, absorption, and lasing distributions in the cross-section of a rubidium cell side-pumped by a LDA are obtained by means of a complicated mathematic procedure. Based on the original end-pumped mode we constructed before, a novel one-direction side-pumped theoretical mode has been established to explore the distribution properties in the transverse section of a rubidium vapor cell by combining the procedures of heat transfer and laser kinetics together. It has been thought the results might be helpful for design of a side-pumped configuration in a high-powered DPAL.

Pre-Excitation Studies for Rubidium-Plasma Generation

CERN Document Server

Aladi, M; Barna, I.F.; Czitrovszky, Aladar; Djotyan, Gagik; Dombi, Peter; Dzsotjan, David; FöLdes, Istvan; Hamar, Gergo; Ignacz, Peter; Kedves, Miklos; Kerekes, Attila; Levai, Peter; Marton, Istvan; Nagy, Attila; Oszetzky, Daniel; Pocsai, Mihaly; Racz, Peter; Raczkevi, Bela; Szigeti, Janos; Sörlei, Zsuzsa; Szipöcs, Robert; Varga, Dezso; Varga-Umbrich, Karoly; Varro, Sandor; Vamos, Lenard; Vesztergombi, György

2014-01-01

The key element in the Proton-Driven-Plasma-Wake-Field-Accelerator (AWAKE) project is the generation of highly uniform plasma from Rubidium vapor. The standard way to achieve full ionization is to use high power laser which can assure the over-barrier-ionization (OBI) along the 10 meters long active region. The Wigner-team in Budapest is investigating an alternative way of uniform plasma generation. The proposed Resonance Enhanced Multi Photon Ionization (REMPI) scheme probably can be realized by much less laser power. In the following the resonant pre-excitations of the Rb atoms are investigated, theoretically and the status report about the preparatory work on the experiment are presented.

Systematic observation of tunneling field-ionization in highly excited Rb Rydberg atoms

International Nuclear Information System (INIS)

Kishimoto, Y.; Tada, M.; Kominato, K.; Shibata, M.; Yamada, S.; Haseyama, T.; Ogawa, I.; Funahashi, H.; Yamamoto, K.; Matsuki, S.

2002-01-01

Pulsed field ionization of high-n (90≤n≤150) manifold states in Rb Rydberg atoms has been investigated in high slew-rate regime. Two peaks in the field ionization spectra were systematically observed for the investigated n region, where the field values at the lower peak do not almost depend on the excitation energy in the manifold, while those at the higher peak increase with increasing excitation energy. The fraction of the higher peak component to the total ionization signals increases with increasing n, exceeding 80% at n=147. Characteristic behavior of the peak component and the comparison with theoretical predictions indicate that the higher peak component is due to the tunneling process. The obtained results show that the tunneling process plays increasingly the dominant role at such highly excited nonhydrogenic Rydberg atoms

Experimental efforts at NIST towards one-electron ions in circular Rydberg states

International Nuclear Information System (INIS)

Tan, Joseph N; Guise, Nicholas D; Brewer, Samuel M

2011-01-01

Experimental effort is underway at NIST to enable tests of theory with one-electron ions synthesized in circular Rydberg states from captured bare nuclei. Problematic effects that limit the accuracy of predicted energy levels for low-lying states are vanishingly small for high-angular-momentum (high-L) states; in particular, the nuclear size correction for high-L states is completely negligible for any foreseeable improvement of measurement precision. As an initial step towards realizing such states, highly charged ions are extracted from the NIST electron beam ion trap (EBIT) and steered through the electrodes of a Penning trap. The goal is to capture bare nuclei in the Penning trap for experiments to make one-electron atoms in circular Rydberg states with dipole (E1) transitions in the optical domain accessible to a frequency comb.

Determination of the Rb atomic number density in dense rubidium vapors by absorption measurements of Rb2 triplet bands

International Nuclear Information System (INIS)

Horvatic, Vlasta; Veza, Damir; Niemax, Kay; Vadla, Cedomil

2008-01-01

A simple and accurate way of determining atom number densities in dense rubidium vapors is presented. The method relies on the experimental finding that the reduced absorption coefficients of the Rb triplet satellite bands between 740 nm and 750 nm and the triplet diffuse band between 600 nm and 610 nm are not temperature dependent in the range between 600 K and 800 K. Therefore, the absolute values of the reduced absorption coefficients of these molecular bands can provide accurate information about atomic number density of the vapor. The rubidium absorption spectrum was measured by spatially resolved white-light absorption in overheated rubidium vapor generated in a heat pipe oven. The absolute values for the reduced absorption coefficients of the triplet bands were determined at lower vapor densities, by using an accurate expression for the reduced absorption coefficient in the quasistatic wing of the Rb D1 line, and measured triplet satellite bands to the resonance wing optical depth ratio. These triplet satellite band data were used to calibrate in absolute scale the reduced absorption coefficients of the triplet diffuse band at higher temperatures. The obtained values for the reduced absorption coefficient of these Rb molecular features can be used for accurate determination of rubidium atomic number densities in the range from about 5 x 10 16 cm -3 to 1 x 10 18 cm -3

Observations of cold antihydrogen

International Nuclear Information System (INIS)

Tan, J.N.; Bowden, N.S.; Gabrielse, G.; Oxley, P.; Speck, A.; Storry, C.H.; Wessels, M.; Grzonka, D.; Oelert, W.; Schepers, G.; Sefzick, T.; Walz, J.; Pittner, H.; Haensch, T.W.; Hessels, E.A.

2004-01-01

ATRAP's e + cooling of p-bar in a nested Penning trap has led to reports of cold H-bar produced during such cooling by the ATHENA and ATRAP collaborations. To observe H-bar, ATHENA uses coincident annihilation detection and ATRAP uses field ionization followed by p-bar storage. Advantages of ATRAP's field ionization method include the complete absence of any background events, and the first way to measure which H-bar states are produced. ATRAP enhances the H-bar production rate by driving many cycles of e + cooling in the nested trap, with more H-bar counted in an hour than the sum of all the other antimatter atoms ever reported. The number of H-bar counted per incident high energy p-bar is also higher than ever observed. The first measured distribution of H-bar states is made using a pre-ionizing electric field between separated production and detection regions. The high rate and the high Rydberg states suggest that the H-bar is formed via three-body recombination, as expected

X-ray and neutron diffraction and molecular dynamics simulation of molten lithium and rubidium nitrates

International Nuclear Information System (INIS)

Yamaguchi, Toshio; Okada, Isao; Ohtaki, Hitoshi; Mikami, Masuhiro; Kawamura, Kazutaka

1986-01-01

Molecular dynamics simulations have been performed for lithium and rubidium nitrate melts at 550 and 600K, respectively, together with X-ray and neutron diffraction experiments. Simple Coulomb pair potentials with Born-type repulsions have been adopted in the simulations with a rigid body model for the nitrate ion. Structure functions derived from the X-ray and neutron experiments are well reproduced by the simulations, from which the three-dimensional cation distribution around the nitrate ion has been revealed. The self-diffusion coefficients, the velocity autocorrelation functions and the self-exchange velocities of lithium, rubidium and nitrate ions have been calculated. Anisotropic motion of nitrate ions has been found and is discussed on the basis of the structure of the melts. (author)

Spin--orbit configuration-interaction study of valence and Rydberg states of LiBe

International Nuclear Information System (INIS)

Marino, M.M.; Ermler, W.C.; Kern, C.W.; Bondybey, V.E.

1992-01-01

Ab initio spin--orbit full configuration-interaction calculations in the context of relativistic effective core potentials are reported for the weakly bound metal dimer LiBe, a three-valence-electron system. The effects of basis set on the energies of valence and Rydberg states of the cluster are discussed, as are the effects of configuration space selection on the energy of the latter states. Results at the dissociative limit are compared to the experimental atomic spectra. Potential-energy curves and spectroscopic constants are presented for the ground state and fourteen excited states, which includes the Li and Be 2p valence states, the Li 3s, 3p, 3d, and 4s Rydberg states, as well as three low-lying states of the molecular cation

Combined theoretical and experimental study of the valence, Rydberg, and ionic states of chlorobenzene

Energy Technology Data Exchange (ETDEWEB)

Palmer, Michael H., E-mail: m.h.palmer@ed.ac.uk; Ridley, Trevor, E-mail: tr01@staffmail.ed.ac.uk, E-mail: vronning@phys.au.dk, E-mail: nykj@phys.au.dk, E-mail: marcello.coreno@elettra.eu, E-mail: desimone@iom.cnr.it, E-mail: malgorzata.biczysko@shu.edu.cn, E-mail: alberto.baiardi@sns.it, E-mail: kipeters@wsu.edu [School of Chemistry, University of Edinburgh, Joseph Black Building, David Brewster Road, Edinburgh EH9 3FJ, Scotland (United Kingdom); Vrønning Hoffmann, Søren, E-mail: tr01@staffmail.ed.ac.uk, E-mail: vronning@phys.au.dk, E-mail: nykj@phys.au.dk, E-mail: marcello.coreno@elettra.eu, E-mail: desimone@iom.cnr.it, E-mail: malgorzata.biczysko@shu.edu.cn, E-mail: alberto.baiardi@sns.it, E-mail: kipeters@wsu.edu; Jones, Nykola C., E-mail: tr01@staffmail.ed.ac.uk, E-mail: vronning@phys.au.dk, E-mail: nykj@phys.au.dk, E-mail: marcello.coreno@elettra.eu, E-mail: desimone@iom.cnr.it, E-mail: malgorzata.biczysko@shu.edu.cn, E-mail: alberto.baiardi@sns.it, E-mail: kipeters@wsu.edu [ISA, Department of Physics and Astronomy, Aarhus University, Ny Munkegade 120, DK-8000 Aarhus C (Denmark); Coreno, Marcello, E-mail: tr01@staffmail.ed.ac.uk, E-mail: vronning@phys.au.dk, E-mail: nykj@phys.au.dk, E-mail: marcello.coreno@elettra.eu, E-mail: desimone@iom.cnr.it, E-mail: malgorzata.biczysko@shu.edu.cn, E-mail: alberto.baiardi@sns.it, E-mail: kipeters@wsu.edu [CNR-ISM, Basovizza Area Science Park, 1-34149 Trieste (Italy); De Simone, Monica, E-mail: tr01@staffmail.ed.ac.uk, E-mail: vronning@phys.au.dk, E-mail: nykj@phys.au.dk, E-mail: marcello.coreno@elettra.eu, E-mail: desimone@iom.cnr.it, E-mail: malgorzata.biczysko@shu.edu.cn, E-mail: alberto.baiardi@sns.it, E-mail: kipeters@wsu.edu [CNR-IOM Laboratorio TASC, Trieste (Italy); Grazioli, Cesare [CNR-IOM Laboratorio TASC, Trieste (Italy); Department of Chemical and Pharmaceutical Sciences, University of Trieste, Trieste (Italy); Zhang, Teng [Department of Physics and Astronomy, University of Uppsala, Uppsala (Sweden); and others

2016-03-28

New photoelectron (PE) and ultra violet (UV) and vacuum UV (VUV) spectra have been obtained for chlorobenzene by synchrotron study with higher sensitivity and resolution than previous work and are subjected to detailed analysis. In addition, we report on the mass-resolved (2 + 1) resonance enhanced multiphoton ionization (REMPI) spectra of a jet-cooled sample. Both the VUV and REMPI spectra have enabled identification of a considerable number of Rydberg states for the first time. The use of ab initio calculations, which include both multi-reference multi-root doubles and singles configuration interaction (MRD-CI) and time dependent density functional theoretical (TDDFT) methods, has led to major advances in interpretation of the vibrational structure of the ionic and electronically excited states. Franck-Condon (FC) analyses of the PE spectra, including both hot and cold bands, indicate much more complex envelopes than previously thought. The sequence of ionic states can be best interpreted by our multi-configuration self-consistent field computations and also by comparison of the calculated vibrational structure of the B and C ionic states with experiment; these conclusions suggest that the leading sequence is the same as that of iodobenzene and bromobenzene, namely: X{sup 2}B{sub 1}(3b{sub 1}{sup −1}) < A{sup 2}A{sub 2}(1a{sub 2}{sup −1}) < B{sup 2}B{sub 2}(6b{sub 2}{sup −1}) < C{sup 2}B{sub 1}(2b{sub 1}{sup −1}). The absorption onset near 4.6 eV has been investigated using MRD-CI and TDDFT calculations; the principal component of this band is {sup 1}B{sub 2} and an interpretation based on the superposition of FC and Herzberg-Teller contributions has been performed. The other low-lying absorption band near 5.8 eV is dominated by a {sup 1}A{sub 1} state, but an underlying weak {sup 1}B{sub 1} state (πσ{sup ∗}) is also found. The strongest band in the VUV spectrum near 6.7 eV is poorly resolved and is analyzed in terms of two ππ{sup ∗} states of

Rydberg dressing of atoms in optical lattices

Science.gov (United States)

Macrı, T.; Pohl, T.

2014-01-01

We study atoms in optical lattices whose electronic ground state is off-resonantly coupled to a highly excited state with strong binary interactions. We present a time-dependent treatment of the resulting quantum dynamics, which—contrary to recent predictions [36 Li, Ates, and Lesanovsky, Phys. Rev. Lett. 110, 213005 (2013), 10.1103/PhysRevLett.110.213005]—proves that the strong repulsion between the weakly admixed Rydberg states does not lead to atomic trap loss. This finding provides an important basis for creating and manipulating coherent long-range interactions in optical lattice experiments.

Long-term evolution and revival structure of Rydberg wave packets

International Nuclear Information System (INIS)

Bluhm, R.

1995-01-01

It is known that, after formation, a Rydberg wave packet undergoes a series of collapses and revivals within a time period called the revival time, t rev , at the end of which it is close to its original shape. We study the behavior of Rydberg wave packets on time scales much greater than t rev . We show that after a few revival cycles the wave packet ceases to reform at multiples of the revival time. Instead, a new series of collapses and revivals commences, culminating after a time period t sr >>t rev with the formation of a wave packet that more closely resembles the initial packet than does the full revival at time t rev . Furthermore, at times that are rational fractions of t sr , the square of the autocorrelation function exhibits large peaks with periodicities that can be expressed as fractions of the revival time t rev . These periodicities indicate a new type of fractional revival occurring for times much greater than t rev . A theoretical explanation of these effects is outlined. ((orig.))

Ionization of Rydberg atoms by the kicks of half-cycle pulses

Indian Academy of Sciences (India)

2015-11-27

Home; Journals; Pramana – Journal of Physics; Volume 86; Issue 4. Ionization of Rydberg atoms by the kicks of half-cycle pulses ... Proceedings of the International Workshop/Conference on Computational Condensed Matter Physics and Materials Science (IWCCMP-2015). Posted on November 27, 2015. Guest Editors: ...

Optimal control of Rydberg lattice gases

Science.gov (United States)

Cui, Jian; van Bijnen, Rick; Pohl, Thomas; Montangero, Simone; Calarco, Tommaso

2017-09-01

We present optimal control protocols to prepare different many-body quantum states of Rydberg atoms in optical lattices. Specifically, we show how to prepare highly ordered many-body ground states, GHZ states as well as some superposition of symmetric excitation number Fock states, that inherit the translational symmetry from the Hamiltonian, within sufficiently short excitation times minimising detrimental decoherence effects. For the GHZ states, we propose a two-step detection protocol to experimentally verify the optimised preparation of the target state based only on standard measurement techniques. Realistic experimental constraints and imperfections are taken into account by our optimisation procedure making it applicable to ongoing experiments.

Optimal control of Rydberg lattice gases

DEFF Research Database (Denmark)

Cui, Jian; Bijnen, Rick van; Pohl, Thomas

2017-01-01

the translational symmetry from the Hamiltonian, within sufficiently short excitation times minimising detrimental decoherence effects. For the GHZ states, we propose a two-step detection protocol to experimentally verify the optimised preparation of the target state based only on standard measurement techniques....... Realistic experimental constraints and imperfections are taken into account by our optimisation procedure making it applicable to ongoing experiments.......We present optimal control protocols to prepare different many-body quantum states of Rydberg atoms in optical lattices. Specifically, we show how to prepare highly ordered many-body ground states, GHZ states as well as some superposition of symmetric excitation number Fock states, that inherit...

Energy redistribution in the dissociation of low Rydberg states of HeH and 02

International Nuclear Information System (INIS)

Zande, W.J.A. van der.

1988-01-01

In this thesis the dissocation process is studied of the diatomic molecules, heliumhydride and molecular oxygen. In ch.'s 2-4 results on the spectroscopy and dissociative decay of the excited states of heliumhydride (HeH) are explained. The positions and dissociation pathways of the A 2 Σ + and B 2 Π states are determined and a theoretical description of the decay of these states are given. An isotope dependent dissociation behaviour of the C 2 /σ + Rydberg state is reported which explained with this theory. In ch.'s 5-7 observations are presented regarding the first Rydberg states of molecular oxygen. The spectroscopy of the (3sσ)d 1 Π g and C 3 Π g states is treated, and the stability and decay of these Rydberg states is discussed qualitatively. An experimental study is described of the (3sσ)d 1 Π g , v=4-8 states. By isotope studies and resolving rotational lines and the measurements of natural linewidths quantitative estimates have been acquired on coupling strengths, positions of repulsive valence states and perturbations reported in literature from REMPI experiments. The electronic coupling strengths between the C 3 Π g state and the 3 Π g valence state has been established. Observed spin-orbit interactions have been quantified and the dissociation of the multiplet states (C 3 Π g , ω=0-2 has been correlated with the multiplet states of the fragment O 3 P J=0-2 . The spectroscopy of the (3sσ3) Rydberg states which con- verge to and are formed in collisions with the O + 2 , a 4 Π μ ion state, is treated. The (3sσ) 5 /π μ state competition between auto-ionizations and (pre-)dissociation has been observed. 207 refs.; 36 figs.; 18 tabs

Quasi-free scattering in the ionization and destruction of hydrogen and helium Rydberg atoms in collision with neutral targets

International Nuclear Information System (INIS)

Renwick, S.P.

1992-01-01

Hydrogen and helium Rydberg atoms (H** and He**), with principal quantum number n ranging from 10 to 20, have been used in collision experiments from 1 to 40 keV/amu. These were produced by electron capture in a charge-exchange cell and analyzed by ionization in a modulated electric field combined with phase-sensitive detection. Three experiments have been conducted. In the first, spectra of the band of H and He Rydberg states from electron capture were produced by the modulated field technique and compared. Considerable differences were found between the two. Both types of spectra were analyzed with calculations of Stark energies and field ionization rates. Attempts were made to simulate the spectra using this information and some assumptions about the state distribution produced in the electron capture. In the second experiment, destruction cross sections for H** incident on N 2 , Ar, and SF 6 were measured. This was a further test of the independent-particle model for Rydberg atom scattering; in this model, the atom is destroyed by quasi-free scattering of either the ionic core or the outer electron. Already proven valid for n = 20-35, this has been extended to n as low as 10, as measurements with n = 10 showed full compliance with the model. In the third experiment, not only destruction cross sections but also ionization cross sections for H** and He** incident on Xe, AR, and N 2 were measured. The ionization measurement is a more sensitive test of the quasi-free scattering of the Rydberg electron. This was especially important for the Xe and Ar targets, which exhibits a Ramsauer-Townsend minimum in their free-electron scattering cross sections. The quasi-free Rydberg electron should reproduce these data. Unmistakable deviations from the quasi-free prediction were seen in Xe and N 2 but not in Ar. This represents the first measurement of a breakdown of the Independent Particle Model for fast Rydberg atom scattering

Measurement of Na-K-ATPase-mediated rubidium influx in single segments of rat nephron

Energy Technology Data Exchange (ETDEWEB)

Cheval, L.; Doucet, A. (Centre National de la Recherche Scientifique, Paris (France))

1990-07-01

To determine the functioning rate of Na-K-ATPase in the rat nephron, a micromethod was developed to measure the rate of rubidium uptake in single nephron segments microdissected from collagenase-treated kidneys. Because the hydrolytic activity of Na-K-ATPase displayed the same apparent affinity for K and Rb ions, whereas the Vmax elicited by K was higher than that in the presence of Rb, experiments were performed in the presence of cold Rb plus 86Rb. Before the assay, tubules were preincubated for 10 min at 37 degrees C to restore the normal transmembrane cation gradients. 86Rb uptake was measured after washing out extracellular cations by rinsing the tubules in ice-cold choline chloride solution containing Ba2+. Rb uptake increased quasi-linearly as a function of incubation time up to 30 s in the thick ascending limb, 1 min in the proximal convoluted tubule, and 5 min in the collecting tubule, and reached an equilibrium after 5-30 min. The initial rates of Rb uptake increased in a saturable fashion as Rb concentration in the medium rose from 0.25 to 5 mM. In medullary thick ascending limb, the initial rate of Rb uptake was inhibited by greater than 90% by 2.5 mM ouabain and by 10(-5) M of the metabolic inhibitor carbonyl cyanide trifluoromethoxyphenylhydrazone. Correlation of Na-K-ATPase hydrolytic activity at Vmax and initial rates of ouabain-sensitive Rb uptake in the successive segments of nephron indicates that in intact cells the pump works at approximately 20-30% of its Vmax. Increasing intracellular Na concentration by tubule preincubation in a Rb- and K-free medium increased the initial rates of Rb intake up to the Vmax of the hydrolytic activity of the pump.

Measurement of Na-K-ATPase-mediated rubidium influx in single segments of rat nephron

International Nuclear Information System (INIS)

Cheval, L.; Doucet, A.

1990-01-01

To determine the functioning rate of Na-K-ATPase in the rat nephron, a micromethod was developed to measure the rate of rubidium uptake in single nephron segments microdissected from collagenase-treated kidneys. Because the hydrolytic activity of Na-K-ATPase displayed the same apparent affinity for K and Rb ions, whereas the Vmax elicited by K was higher than that in the presence of Rb, experiments were performed in the presence of cold Rb plus 86Rb. Before the assay, tubules were preincubated for 10 min at 37 degrees C to restore the normal transmembrane cation gradients. 86Rb uptake was measured after washing out extracellular cations by rinsing the tubules in ice-cold choline chloride solution containing Ba2+. Rb uptake increased quasi-linearly as a function of incubation time up to 30 s in the thick ascending limb, 1 min in the proximal convoluted tubule, and 5 min in the collecting tubule, and reached an equilibrium after 5-30 min. The initial rates of Rb uptake increased in a saturable fashion as Rb concentration in the medium rose from 0.25 to 5 mM. In medullary thick ascending limb, the initial rate of Rb uptake was inhibited by greater than 90% by 2.5 mM ouabain and by 10(-5) M of the metabolic inhibitor carbonyl cyanide trifluoromethoxyphenylhydrazone. Correlation of Na-K-ATPase hydrolytic activity at Vmax and initial rates of ouabain-sensitive Rb uptake in the successive segments of nephron indicates that in intact cells the pump works at approximately 20-30% of its Vmax. Increasing intracellular Na concentration by tubule preincubation in a Rb- and K-free medium increased the initial rates of Rb intake up to the Vmax of the hydrolytic activity of the pump

Accurate Mapping of Multilevel Rydberg Atoms on Interacting Spin-1 /2 Particles for the Quantum Simulation of Ising Models

Science.gov (United States)

de Léséleuc, Sylvain; Weber, Sebastian; Lienhard, Vincent; Barredo, Daniel; Büchler, Hans Peter; Lahaye, Thierry; Browaeys, Antoine

2018-03-01

We study a system of atoms that are laser driven to n D3 /2 Rydberg states and assess how accurately they can be mapped onto spin-1 /2 particles for the quantum simulation of anisotropic Ising magnets. Using nonperturbative calculations of the pair potentials between two atoms in the presence of electric and magnetic fields, we emphasize the importance of a careful selection of experimental parameters in order to maintain the Rydberg blockade and avoid excitation of unwanted Rydberg states. We benchmark these theoretical observations against experiments using two atoms. Finally, we show that in these conditions, the experimental dynamics observed after a quench is in good agreement with numerical simulations of spin-1 /2 Ising models in systems with up to 49 spins, for which numerical simulations become intractable.

The role of high Rydberg states in the generation of negative ions in negative-ion discharges

International Nuclear Information System (INIS)

Hiskes, J.R.

1995-01-01

The generation of substantial yields of H - ions in a laser excited H 2 gas has been reported by Pinnaduwage and Christoforu. These H - yields have been attributed to (2 + 1) REMP photoexcitation processes leading to dissociative attachment of doubly-excited or superexcited states (SES), or dissociative attachment of high Rydberg product states. The new feature of these experiments is the implied large dissociative attachment rates, of order 10 -6 cm 3 sec -1 , values that are orders-of-magnitude larger than the dissociative attachment of the vibrationally excited levels of the ground electronic state. While these laser excitations are not directly applicable to a hydrogen negative-ion discharge, the implication of large dissociative attachment rates to the high Rydberg states may affect both the total negative-ion density and the interpretation of discharge performance. Within the discharge energetic electrons will collisionally excite the higher Rydberg states, and the relative contribution of the dissociative attachment of these states when compared with the dissociative attachment to the ground state vibrational levels, is the topic of this paper

Effects of confinement on the Rydberg molecule NeH

International Nuclear Information System (INIS)

Lo, J M H; Klobukowski, M; Bielinska-Waz, D; Diercksen, G H F; Schreiner, E W S

2005-01-01

Ab initio potential energy curves of the Rydberg NeH molecule in the presence of cylindrical spatial confinement were computed by the method of multi-reference configuration interaction with extended basis sets. The influence of the applied potential to the structures and spectra of the ground and excited states of NeH was analysed in terms of perturbation theory. In addition, the phenomenon of field-induced ionization was discussed

Labeling Feral Spruce Budworm (Lepidoptera: Tortricidae) Populations With Rubidium.

Science.gov (United States)

MacKinnon, Wayne; Eveleigh, Eldon; Silk, Peter; Forbes, Glen

2016-04-01

Rubidium (Rb) is a trace element that occurs naturally in low concentrations and is easily absorbed by plants, making it a useful tool for labeling insect defoliators, such as spruce budworm (Choristoneura fumiferana Clemens). Balsam fir trees (Abies balsamea (L.) Miller) injected with either 8 or 16 g per tree of rubidium chloride (RbCl) showed quick uptake and distribution throughout the crown, with no negative effects on tree shoot growth or spruce budworm survival and development. Adult spruce budworm that fed as larvae on trees injected with RbCl were clearly labeled, with significantly higher Rb concentrations than the background levels found in adults that fed as larvae on control trees. Rb concentrations in feral spruce budworm adults for both the 8 g (9 µg/g) and 16 g (25 µg/g) per tree treatments were at least five times lower than those in laboratory-reared adults on 1,000 µg/g RbCl diet (125 µg/g); survival, development, pupal weight, sex ratio, and mating status of spruce budworm were not adversely affected by Rb treatment. Egg masses laid by feral females that fed as larvae on Rb-labeled trees were also labeled with Rb. Injecting trees with RbCl is a viable technique for labeling feral spruce budworm populations to help distinguish local populations from immigrants to better evaluate the success of early intervention strategies such as mating disruption. © Crown copyright 2016.

Properties of Ni^+ from microwave spectroscopy of n=9 Rydberg levels of Nickel

Science.gov (United States)

Woods, Shannon; Keele, Julie; Smith, Chris; Lundeen, Stephen

2012-06-01

The microwave/RESIS method was used to determine the relative positions of 15 of the n=9 Rydberg levels of Nickel with L >= 6. Because the ground state of the Ni^+ ion is a ^2D5/2 level, each Rydberg level (n,L) splits into six eigenstates whose relative positions are determined by long-range e-Ni^+ interactions present in addition to the dominant Coulomb interaction. A previous study with the optical RESIS method determined these positions with precision of +/- 30 MHz [1]. Using the microwave/RESIS method improves that precision by a factor of 300, and leads to much improved determinations of the Ni+ properties that control the long-range interactions. [4pt] [1] Julie A. Keele, Shannon L. Woods, M.E. Hanni, and S.R. Lundeen Phys. Rev. 81, 022506 (2010)

Recent results of the pulsed optically pumped rubidium clock

Science.gov (United States)

Levi, F.; Micalizio, S.; Godone, A.; Calosso, C.; Bertacco, E.

2017-11-01

A laboratory prototype of a pulsed optically pumped (POP) clock based on a rubidium cell with buffer gas is described. This clock has shown very interesting physical and metrological features, such as negligible light-shift, strongly reduced cavity-pulling and very good frequency stability. In this regard, an Allan deviation of σy(τ) = 1.2 τ-1/2 for measurement times up to τ = 105 s has been measured. These results confirm the interesting perspectives of such a frequency standard and make it very attractive for several technological applications, such as radionavigation.

Rydberg atoms in weak magnetic fields

International Nuclear Information System (INIS)

Kazantsev, A.P.; Pokrovsky, V.L.; Bergou, J.

1983-01-01

The quadratic Zeeman effect of Rydberg atoms in the framework of perturbation theory is dealt with and a special quasiclassical approximation scheme is applied. The Bohr-Sommerfeld quantization condition is given in terms of complete elliptic integrals. It is shown that part of the spectrum is doubly degenerate, the corresponding states are asymmetric with respect to the Coulomb centre and have a non-zero dipole moment; the rest of the spectrum is nondegenerate, the states are symmetric and their dipole-moment vanishes. The transition from the symmetric to the asymmetric region is similar to a phase transition and it gives an experimental possibility to distinguish between the two types of states. (author)

Microwave-to-optical frequency conversion with a Rydberg atom coupled to a coplanar waveguide

Science.gov (United States)

Gard, Bryan; Jacobs, Kurt; McDermott, Robert; Saffman, Mark

2017-04-01

A primary candidate for converting quantum information from microwave to optical frequencies is the use of Rydberg states of a single atom trapped near a surface. The fact that the Rydberg states possess both large electric dipole moments and microwave transition frequencies allows them to interact with superconducting mesoscopic circuits. By considering a concrete example, that of a Cesium atom, and using numerical search methods to optimize the control protocols, we determine the fidelities and transmission rates that could be achievable with such a device. We show that while protocols that exploit the adiabatic STIRAP mechanism provide the best raw transfer fidelities, the fastest communication speeds can be obtained by using heralding, which allows one to remove the adiabatic constraint. Support from Oak Ridge Associated Universities.

Optical potential study of electron scattering by rubidium

Energy Technology Data Exchange (ETDEWEB)

Chin, J. H.; Ratnavelu, K. [University of Malaya, Kuala Lumpur (Malaysia); Zhou, Y. [Harbin Institute of Technology, Harbin (China)

2011-10-15

The coupled-channel optical method (CCOM) has been implemented in a study of electronrubidium scattering. This method includes the continuum effect in the calculation via an ab-initio optical potential. Eight atomic states (5s, 5p, 4d, 6s, 6p, 5d, 7s, 7p) were used together with the continuum optical potential in the 5s-5s, 5s-5p, and 5p-5p coupling. The elastic, inelastic and total cross sections for electron-rubidium scattering at low and intermediate energies, ranging from 10 eV to 100 eV, are reported. The results are compared with available experimental and theoretical data.

Hybrid Systems: Cold Atoms Coupled to Micro Mechanical Oscillators =

Science.gov (United States)

Montoya Monge, Cris A.

Micro mechanical oscillators can serve as probes in precision measurements, as transducers to mediate photon-phonon interactions, and when functionalized with magnetic material, as tools to manipulate spins in quantum systems. This dissertation includes two projects where the interactions between cold atoms and mechanical oscillators are studied. In one of the experiments, we have manipulated the Zeeman state of magnetically trapped Rubidium atoms with a magnetic micro cantilever. The results show a spatially localized effect produced by the cantilever that agrees with Landau-Zener theory. In the future, such a scalable system with highly localized interactions and the potential for single-spin sensitivity could be useful for applications in quantum information science or quantum simulation. In a second experiment, work is in progress to couple a sample of optically trapped Rubidium atoms to a levitated nanosphere via an optical lattice. This coupling enables the cooling of the center-of-mass motion of the nanosphere by laser cooling the atoms. In this system, the atoms are trapped in the optical lattice while the sphere is levitated in a separate vacuum chamber by a single-beam optical tweezer. Theoretical analysis of such a system has determined that cooling the center-of-mass motion of the sphere to its quantum ground state is possible, even when starting at room temperature, due to the excellent environmental decoupling achievable in this setup. Nanospheres cooled to the quantum regime can provide new tests of quantum behavior at mesoscopic scales and have novel applications in precision sensing.

A heated vapor cell unit for DAVLL in atomic rubidium

OpenAIRE

McCarron, Daniel J.; Hughes, Ifan G.; Tierney, Patrick; Cornish, Simon L.

2007-01-01

The design and performance of a compact heated vapor cell unit for realizing a dichroic atomic vapor laser lock (DAVLL) for the D2 transitions in atomic rubidium is described. A 5 cm-long vapor cell is placed in a double-solenoid arrangement to produce the required magnetic field; the heat from the solenoid is used to increase the vapor pressure and correspondingly the DAVLL signal. We have characterized experimentally the dependence of important features of the DAVLL signal on magnetic field...

Studies on alterations of the 86-rubidium efflux from rat pancreatic islets caused by thiol and thiol oxidants

International Nuclear Information System (INIS)

Wahl, M.A.

1983-01-01

The following findings were revealed by this study: 1) Oxidation-reduction (redox) of the intracellular system of glutathione influences the potassium efflux by way of an increase in the 86-rubidium efflux brought about by the oxidation of intracellular thiols. 2) The 86-rubidium efflux is not subject to change by oxidation of extracellular thiols located in the membrane, nor can it in any way be influenced by reduced glutathione of exogenous origin. 3) The potassium efflux from rat pancreatic islets, being generally known to trigger the electric activities of the beta-cell, is controlled by the oxidation-reduction of intracellular thiols rather than by that of extracellular thiols. (TRV) [de

Laser pulse propagation in a meter scale rubidium vapor/plasma cell in AWAKE experiment

Energy Technology Data Exchange (ETDEWEB)

Joulaei, A. [Max-Planck Institute for Physics, Munich (Germany); University of Mazandaran (Iran, Islamic Republic of); Moody, J. [Max-Planck Institute for Physics, Munich (Germany); Berti, N.; Kasparian, J. [University of Geneva (Switzerland); Mirzanejhad, S. [University of Mazandaran (Iran, Islamic Republic of); Muggli, P. [Max-Planck Institute for Physics, Munich (Germany)

2016-09-01

We present the results of numerical studies of laser pulse propagating in a 3.5 cm Rb vapor cell in the linear dispersion regime by using a 1D model and a 2D code that has been modified for our special case. The 2D simulation finally aimed at finding laser beam parameters suitable to make the Rb vapor fully ionized to obtain a uniform, 10 m-long, at least 1 mm in radius plasma in the next step for the AWAKE experiment. - Highlights: • Discussion the AWAKE plasma source based on photoionization of rubidium vapor with a TW/cm^2 Intensity laser with a spectrum across valence ground state transition resonances. • Examines the propagation of the AWAKE ionization laser through rubidium vapor at design density on a small scale and reduced intensity with a linear numerical model compared to experimental results. • Discusses physics of pulse propagation through the vapor at high intensity regime where strong ionization occurs within the laser pulse.

Rydberg atoms in circular polarization: Classical stabilization in optical frequency fields

International Nuclear Information System (INIS)

Chism, Will; Reichl, L.E.

2002-01-01

We investigate the classical dynamics of the Rydberg atom in circularly polarized laser fields, restricted to the two-dimensional plane of polarization. We use a Poincare surface of section to study nonlinear resonance structures for optical frequency driving fields. We demonstrate the existence and morphology of these structures as the laser intensity transitions from moderate to intense

Asymptotics of Rydberg states for the hydrogen atom

International Nuclear Information System (INIS)

Thomas, L.E.

1997-01-01

The asymptotics of Rydberg states, i.e., highly excited bound states of the hydrogen atom Hamiltonian, and various expectations involving these states are investigated. We show that suitable linear combinations of these states, appropriately rescaled and regarded as functions either in momentum space or configuration space, are highly concentrated on classical momentum space or configuration space Kepler orbits respectively, for large quantum numbers. Expectations of momentum space or configuration space functions with respect to these states are related to time-averages of these functions over Kepler orbits. (orig.)

The kicked Rydberg atom: Regular and stochastic motion

International Nuclear Information System (INIS)

Burgdoerfer, J.

1988-01-01

We have investigated the dynamics of a three-dimensional classical Rydberg atom driven by a sequence of pulses. Both the deterministic system with periodic pulses and the closely related ''noisy'' system with random pulses have been studied in parallel. The Lyapunov exponent is calculated as a function of pulse height and the angular momentum of the initial state. We find differences between noisy and deterministic perturbations to be most pronounced for small pulse heights. Low angular momentum orbits show enhanced diffusion in agreement with recent experimental data for ion-solid interaction. 22 refs., 6 figs

Crystal structure of rubidium methyldiazotate

Directory of Open Access Journals (Sweden)

Tobias Grassl

2017-02-01

Full Text Available The title compound, Rb+·H3CN2O−, has been crystallized in liquid ammonia as a reaction product of the reductive ammonolysis of the natural compound streptozocin. Elemental rubidium was used as reduction agent as it is soluble in liquid ammonia, forming a blue solution. Reductive bond cleavage in biogenic materials under kinetically controlled conditions offers a new approach to gain access to sustainably produced raw materials. The anion is nearly planar [dihedral angle O—N—N—C = −0.4 (2°]. The Rb+ cation has a coordination number of seven, and coordinates to five anions. One anion is bound via both its N atoms, one by both O and N, two anions are bound by only their O atoms, and the last is bound via the N atom adjacent to the methyl group. The diazotate anions are bridged by cations and do not exhibit any direct contacts with each other. The cations form corrugated layers that propagate in the (-101 plane.

Low-temperature phase transformation in rubidium and cesium superoxides

International Nuclear Information System (INIS)

Alikhanov, R.A.; Toshich, B.S.; Smirnov, L.S.

1980-01-01

Crystal structures of rubidium and cesium superoxides which are two interpenetrating lattices of metal ions and oxygen molecule ions reveal a number of phase transformations with temperature decrease. Crystal-phase transformations in CsO 2 are 1-2, 2-3 and low temperature one 3-4 at 378, 190 and 10 K. Low temperature transition is considered as the instability of lattice quadrupoles of oxygen molecule ions to phase transformation of the order-disorder type. Calculated temperatures of low temperature phase transformations in PbO 2 and CsO 2 agree with experimental calculations satisfactory [ru

Improving Rydberg Excitations within Time-Dependent Density Functional Theory with Generalized Gradient Approximations: The Exchange-Enhancement-for-Large-Gradient Scheme.

Science.gov (United States)

Li, Shaohong L; Truhlar, Donald G

2015-07-14

Time-dependent density functional theory (TDDFT) with conventional local and hybrid functionals such as the local and hybrid generalized gradient approximations (GGA) seriously underestimates the excitation energies of Rydberg states, which limits its usefulness for applications such as spectroscopy and photochemistry. We present here a scheme that modifies the exchange-enhancement factor to improve GGA functionals for Rydberg excitations within the TDDFT framework while retaining their accuracy for valence excitations and for the thermochemical energetics calculated by ground-state density functional theory. The scheme is applied to a popular hybrid GGA functional and tested on data sets of valence and Rydberg excitations and atomization energies, and the results are encouraging. The scheme is simple and flexible. It can be used to correct existing functionals, and it can also be used as a strategy for the development of new functionals.

Photoabsorption spectra of potassium and rubidium near the K-edge

International Nuclear Information System (INIS)

Azuma, Y.; Berry, H.G.; Cowan, P.L.

1995-01-01

We have used a high-temperature circulating heat-pipe absorption cell together with monochromatized X-ray beams at the X24A and X23A2 beam lines at the NSLS to obtain photoabsorption spectra of potassium and rubidium at their K- and KM-edges. The photon-energy ranges lay near 3600 eV and 15200 eV, respectively. We have also obtained first measurements of the LII and LIII edges in cesium. Although the K-edge photoabsorptions of the rare gases have been studied, there is little previous work on other atomic vapors. Most of the edges and resonance peaks that we observed have now been identified using Dirac Hartree-Fock calculations. As a check, we have compared these results with those obtained previously in closed-shell rare-gas absorption spectra. The absolute energies were obtained through a calibration of the X24A systems using measurements of several metal L-edges in the 3200-5000 eV energy range. We found that the 4p resonance in potassium is significantly enhanced compared with the corresponding situation in argon. Likewise, the 5p resonance in krypton is unresolved from the background ionization cross section, whereas it is well resolved in rubidium. As suggested by Amusia, these enhancements may be due to the enhanced potential seen in the excited state of the alkali systems as a result of the presence of an s-electron which reduces the nuclear shielding

Orthogonal flexible Rydberg aggregates

Science.gov (United States)

Leonhardt, K.; Wüster, S.; Rost, J. M.

2016-02-01

We study the link between atomic motion and exciton transport in flexible Rydberg aggregates, assemblies of highly excited light alkali-metal atoms, for which motion due to dipole-dipole interaction becomes relevant. In two one-dimensional atom chains crossing at a right angle adiabatic exciton transport is affected by a conical intersection of excitonic energy surfaces, which induces controllable nonadiabatic effects. A joint exciton-motion pulse that is initially governed by a single energy surface is coherently split into two modes after crossing the intersection. The modes induce strongly different atomic motion, leading to clear signatures of nonadiabatic effects in atomic density profiles. We have shown how this scenario can be exploited as an exciton switch, controlling direction and coherence properties of the joint pulse on the second of the chains [K. Leonhardt et al., Phys. Rev. Lett. 113, 223001 (2014), 10.1103/PhysRevLett.113.223001]. In this article we discuss the underlying complex dynamics in detail, characterize the switch, and derive our isotropic interaction model from a realistic anisotropic one with the addition of a magnetic bias field.

Quantum delayed-choice experiment with a single neutral atom.

Science.gov (United States)

Li, Gang; Zhang, Pengfei; Zhang, Tiancai

2017-10-01

We present a proposal to implement a quantum delayed-choice (QDC) experiment with a single neutral atom, such as a rubidium or cesium atom. In our proposal, a Ramsey interferometer is adopted to observe the wave-like or particle-like behaviors of a single atom depending on the existence or absence of the second π/2-rotation. A quantum-controlled π/2-rotation on target atom is realized through a Rydberg-Rydberg interaction by another ancilla atom. It shows that a heavy neutral atom can also have a morphing behavior between the particle and the wave. The realization of the QDC experiment with such heavy neutral atoms not only is significant to understand the Bohr's complementarity principle in matter-wave and matter-particle domains but also has great potential on the quantum information process with neutral atoms.

Ultrafast non-adiabatic dynamics of methyl substituted ethylenes: The π3s Rydberg state

Science.gov (United States)

Wu, Guorong; Boguslavskiy, Andrey E.; Schalk, Oliver; Schuurman, Michael S.; Stolow, Albert

2011-10-01

Excited state unimolecular reactions of some polyenes exhibit localization of their dynamics at a single ethylenic double bond. Here we present studies of the fundamental photophysical processes in the ethylene unit itself. Combined femtosecond time-resolved photoelectron spectroscopy (TRPES) and ab initio quantum chemical calculations was applied to the study of excited state dynamics in cis-butene, trans-butene, trimethylethylene, and tetramethylethylene, following initial excitation to their respective π3s Rydberg states. The wavelength dependence of the π3s Rydberg state dynamics of tetramethylethylene was investigated in more detail. The π3s Rydberg to ππ* valence state decay rate varies greatly with substituent: the 1,2-di- and tri-methyl substituted ethylenes (cis-butene, trans-butene, and trimethylethylene) show an ultrafast decay (˜20 fs), whereas the fully methylated tetramethylethylene shows a decay rate of 2 to 4 orders of magnitude slower. These observations are rationalized in terms of topographical trends in the relevant potential energy surfaces, as found from ab initio calculations: (1) the barrier between the π3s state and the ππ* state increases with increasing methylation, and (2) the π3s/ππ* minimum energy conical intersection displaces monotonically away from the π3s Franck-Condon region with increasing methylation. The use of systematic methylation in combination with TRPES and ab initio computation is emerging as an important tool in discerning the excited state dynamics of unsaturated hydrocarbons.

One step beyond the electric dipole approximation: An experiment to observe the 5p → 6p forbidden transition in atomic rubidium

Science.gov (United States)

Ponciano-Ojeda, F.; Hernández-Gómez, S.; Mojica-Casique, C.; Ruiz-Martínez, E.; López-Hernández, O.; Colín-Rodríguez, R.; Ramírez-Martínez, F.; Flores-Mijangos, J.; Sahagún, D.; Jáuregui, R.; Jiménez-Mier, J.

2018-01-01

An advanced undergraduate experiment to study the 5 P 3 / 2 → 6 P 3 / 2 electric quadrupole transition in rubidium atoms is presented. The experiment uses two external cavity diode lasers, one operating at the D2 rubidium resonance line and the other built with commercial parts to emit at 911 nm. The lasers produce the 5 s → 5 p → 6 p excitation sequence in which the second step is the forbidden transition. Production of atoms in the 6 P 3 / 2 state is observed by detection of the 420 nm fluorescence that results from electric dipole decay into the ground state. Lines whose widths are significantly narrower than the Doppler width are used to study the hyperfine structure of the 6 P 3 / 2 state in rubidium. The spectra illustrate characteristics unique to electric dipole forbidden transitions, like the electric quadrupole selection rules; they are also used to show general aspects of two-color laser spectroscopy such as velocity selection and hyperfine pumping.

A universal representation of Rydberg spectral line shapes in plasmas

International Nuclear Information System (INIS)

Mosse, C.; Calisti, A.; Stamm, R.; Talin, B.; Bureyeva, L.; Lisitsa, V. S.

2001-01-01

A universal representation of Rydberg atom line shapes in plasmas is obtained. It bases on analytical formulas for intensity distribution in radiation transitions n→n' between highly excited atomic states with large values of principle quantum numbers n, n'>>1, Δn=n-n'<< n and the frequency fluctuation model (FFM) for account of ion thermal motion effects. The line shapes are presented in a universal manner as functions of plasma temperatures and densities

Lamb shift of Rydberg atoms in a resonator

International Nuclear Information System (INIS)

Belov, A.A.; Lozovik, Yu.E.; Pokrovsky, V.L.

1988-08-01

The Lamb shift of a Rydberg atom in a cavity is shown to be enhanced with the resonance interaction of a virtual atomic transition and cavity modes. The dependence of the Lamb shift on quantum numbers and atomic number changes drastically. Shifting cavity walls and scanning the atomic beam one can vary the Lamb shift. The value of the Lamb shift in a cavity may exceed a typical magnitude of the fine structure energy. For a rough resonance tuning the Coulumb multiplet occurs to be strongly mixed and a novel classification is necessary. (author). 8 refs, 2 figs

Mesoscopic Rydberg Gate Based on Electromagnetically Induced Transparency

International Nuclear Information System (INIS)

Mueller, M.; Lesanovsky, I.; Zoller, P.; Weimer, H.; Buechler, H. P.

2009-01-01

We demonstrate theoretically a parallelized C-NOT gate which allows us to entangle a mesoscopic ensemble of atoms with a single control atom in a single step, with high fidelity and on a microsecond time scale. Our scheme relies on the strong and long-ranged interaction between Rydberg atoms triggering electromagnetically induced transparency. By this we can robustly implement a conditional transfer of all ensemble atoms between two logical states, depending on the state of the control atom. We outline a many-body interferometer which allows a comparison of two many-body quantum states by performing a measurement of the control atom.

Adiabatic potential-energy curves of long-range Rydberg molecules: Two-electron R -matrix approach

Czech Academy of Sciences Publication Activity Database

Tarana, Michal; Čurík, Roman

2016-01-01

Roč. 93, č. 1 (2016), 012515 ISSN 0556-2791 R&D Projects: GA ČR(CZ) GP14-15989P Institutional support: RVO:61388955 Keywords : adiabatic-potential- energy curves * Rydberg molecules * theoretical chemistry Subject RIV: CF - Physical ; Theoretical Chemistry

Adiabatic potential-energy curves of long-range Rydberg molecules: Two-electron R -matrix approach

Czech Academy of Sciences Publication Activity Database

Tarana, Michal; Čurík, Roman

2016-01-01

Roč. 93, č. 1 (2016), 012515 ISSN 0556-2791 R&D Projects: GA ČR(CZ) GP14-15989P Institutional support: RVO:61388955 Keywords : adiabatic-potential-energy curves * Rydberg molecules * theoretical chemistry Subject RIV: CF - Physical ; Theoretical Chemistry

Dielectric dispersion in pure and doped lithium rubidium sulphate

Science.gov (United States)

Kassem, M. E.; El-Muraikhi, M.; Al-Houty, L.; Mohamed, A. A.

The frequency (102 - 105 Hz) dependence of the dielectric properties of lithium rubidium sulphate (LRS) are reported in the vicinity of the transition temperature Tc = 477 K. The a.c. conductivity σ(ω) shows a strong temperature dependence and weak frequency response. The dielectric constant in this region shows a strong frequency dispersion. A Cole-Cole diagram was used to determine the distribution parameter and the molecular relaxation time. The effect of doping with Dy+3, Sm+3 and V+3, was also studied. It was found that doping gives rise to localized states which produce a disorder in the structure of LiRbSO4.

Crystal structure of rubidium peroxide ammonia disolvate

Directory of Open Access Journals (Sweden)

Tobias Grassl

2017-02-01

Full Text Available The title compound, Rb2O2·2NH3, has been obtained as a reaction product of rubidium metal dissolved in liquid ammonia and glucuronic acid. As a result of the low-temperature crystallization, a disolvate was formed. To our knowledge, only one other solvate of an alkali metal peroxide is known: Na2O2·8H2O has been reported by Grehl et al. [Acta Cryst. (1995, C51, 1038–1040]. We determined the peroxide bond length to be 1.530 (11 Å, which is in accordance with the length reported by Bremm & Jansen [Z. Anorg. Allg. Chem. (1992, 610, 64–66]. One of the ammonia solvate molecules is disordered relative to a mirror plane, with 0.5 occupancy for the corresponding nitrogen atom.

Feshbach resonances in cold collisions of potassium atoms

International Nuclear Information System (INIS)

Bambini, A.; Geltman, S.

2002-01-01

In this paper we briefly review the basic steps that allow the calculation of the scattering length in the collision of two alkali-metal atoms in a well defined magnetic polarization state, and in the presence of a static magnetic field. Calculations are actually done for the low-field seeking state F=1, μ F =-1 of bosonic potassium atoms. The electrostatic potentials obtained through Rydberg-Klein-Rees data are connected to a dispersive, long range tail in which the dominant dipole-dipole C 6 term may take different values within a specified range. We show the occurrence of Feshbach resonances in the ultra cold collision of two identical atoms, belonging either to the bosonic species 39 K or 41 K. Our results demonstrate that there is a range of C 6 values for which the collision of two 39 K atoms displays a single resonance, while for other values of C 6 no resonance occurs. On the other hand, Feshbach resonances are present in the collision of two 41 K atoms for almost all values of the dispersion coefficient C 6 in that range. We also show the origin of the different types of Feshbach resonances that occur in the cold collision of two 41 K atoms. The detection of such resonances can help establish the actual value of the dispersive coefficient

Optical spectroscopy of high-L Rydberg states of argon

International Nuclear Information System (INIS)

Wright, L. E.; Snow, E. L.; Lundeen, S. R.; Sturrus, W. G.

2007-01-01

High-L fine structure patterns in n=9 and n=17 Rydberg levels of argon have been studied using a Doppler-tuned CO 2 laser and a fast beam of argon atoms. Analysis of the measured pattern using the polarization model yields the scalar dipole polarizability and quadrupole moment of the 2 P 3 at ∼sol∼ at 2 Ar + ion. The results are α S =6.83(8)a 0 3 and Q=-0.5177(15)ea 0 2 . Within the precision of this study, no vector component of the structure was observed

Polyatomic Trilobite Rydberg Molecules in a Dense Random Gas.

Science.gov (United States)

Luukko, Perttu J J; Rost, Jan-Michael

2017-11-17

Trilobites are exotic giant dimers with enormous dipole moments. They consist of a Rydberg atom and a distant ground-state atom bound together by short-range electron-neutral attraction. We show that highly polar, polyatomic trilobite states unexpectedly persist and thrive in a dense ultracold gas of randomly positioned atoms. This is caused by perturbation-induced quantum scarring and the localization of electron density on randomly occurring atom clusters. At certain densities these states also mix with an s state, overcoming selection rules that hinder the photoassociation of ordinary trilobites.

Emission characteristics of plasma based on xenon-rubidium bromide mixture

Science.gov (United States)

Heneral, A. A.; Avtaeva, S. V.

2017-10-01

Luminescence spectra of a longitudinal pulse-periodic discharge in xenon mixture with rubidium bromide vapors (Xe-RbBr) are studied experimentally at low pressures. The conditions leading to the appearance of intense bands of ultraviolet radiation of exciplex XeBr* molecules in the spectral interval between 200 and 400 nm are found. The highest yield of UV radiation of XeBr* molecules is achieved when the temperature of discharge-tube walls is equal to 750°C. A maximum power of UV radiation from the entire plasma volume as high as 4.8 W is obtained.

Rydberg-atom based radio-frequency electrometry using frequency modulation spectroscopy in room temperature vapor cells.

Science.gov (United States)

Kumar, Santosh; Fan, Haoquan; Kübler, Harald; Jahangiri, Akbar J; Shaffer, James P

2017-04-17

Rydberg atom-based electrometry enables traceable electric field measurements with high sensitivity over a large frequency range, from gigahertz to terahertz. Such measurements are particularly useful for the calibration of radio frequency and terahertz devices, as well as other applications like near field imaging of electric fields. We utilize frequency modulated spectroscopy with active control of residual amplitude modulation to improve the signal to noise ratio of the optical readout of Rydberg atom-based radio frequency electrometry. Matched filtering of the signal is also implemented. Although we have reached similarly, high sensitivity with other read-out methods, frequency modulated spectroscopy is advantageous because it is well-suited for building a compact, portable sensor. In the current experiment, ∼3 µV cm-1 Hz-1/2 sensitivity is achieved and is found to be photon shot noise limited.

Molecular physics. Production of trilobite Rydberg molecule dimers with kilo-Debye permanent electric dipole moments.

Science.gov (United States)

Booth, D; Rittenhouse, S T; Yang, J; Sadeghpour, H R; Shaffer, J P

2015-04-03

Permanent electric dipole moments are important for understanding symmetry breaking in molecular physics, control of chemical reactions, and realization of strongly correlated many-body quantum systems. However, large molecular permanent electric dipole moments are challenging to realize experimentally. We report the observation of ultralong-range Rydberg molecules with bond lengths of ~100 nanometers and kilo-Debye permanent electric dipole moments that form when an ultracold ground-state cesium (Cs) atom becomes bound within the electronic cloud of an extended Cs electronic orbit. The electronic character of this hybrid class of "trilobite" molecules is dominated by degenerate Rydberg manifolds, making them difficult to produce by conventional photoassociation. We used detailed coupled-channel calculations to reproduce their properties quantitatively. Our findings may lead to progress in ultracold chemistry and strongly correlated many-body physics. Copyright © 2015, American Association for the Advancement of Science.

Electromagnetically induced two-photon transparency in rubidium atoms

International Nuclear Information System (INIS)

Wang, D.; Gao, J.Y.; Xu, J.H.; Bassani, F.; La Rocca, G.C.; Salerno Univ.

2001-01-01

We present an experimental demonstration of electromagnetically induced two-photon transparency (EITT) in room temperature rubidium vapor. The 8S 1/2 to 5P 1/2 fluorescence is used to monitor the 5S 1/2 (F = 3) to 8S 1/2 (F = 3) two-photon absorption near resonance with the intermediate state 5P 3/2 . A controlling pump laser beam is employed to coherently couple the 5P 3/2 and 5D 5/2 states, thus producing two dressed intermediate states which give rise to destructive interference in the two-photon transition. An induced two-photon transparency of about 80% has been obtained at resonance; our experimental findings are in good agreement with the general theory of Agarwal et al. (1996), when the appropriate spectroscopic parameters are used. (orig.)

Przebieg mitozy w korzeniach siewek pszenicy pod wpływem rubidu [Course of mitosis in root seedlings of Triticum aestivum L. under the influence of rubidium

Directory of Open Access Journals (Sweden)

Kazimierz Olech

2015-06-01

Full Text Available The depresion of mitosis as a result of rubidium action illustrated by the lower frequency of mitosis was found in an investigation made on roots of wheat seedlings grown on a nutrient medium which the total amount of potassium or a half of it was replaced by rubidium. The lower mitotic activity was caused by limited number of nuclei beginning prophase and by a prolonged duration of metaphase.

Strongly perturbed Rydberg series originating from KrII 4p45s ionic states

International Nuclear Information System (INIS)

Petrov, I.D.; Demekhin, Ph.V.; Lagutin, B.M.; Sukhorukov, V.L.; Kammer, S.; Mickat, S.; Schartner, K.-H.; Ehresmann, A.; Klumpp, S.; Werner, L.; Schmoranzer, H.

2005-01-01

Photoionization cross-sections for the 4p 4 ( 3 P) 5s 4 P 5/2,3/2,1/2 satellites and 4s, 4p main levels of Kr II in the exciting-photon energy range between 28.48 and 28.70-bar eV with extremely narrow bandwidth (1.7-bar meV at 28.55-bar eV) of the monochromatized synchrotron radiation were measured utilizing the photon-induced fluorescence spectroscopy. The observed resonances were assigned to the 4p 4 5s( 4 P 1/2 )n p and 4p 4 5s( 2 P 3/2 )n p Rydberg series on the basis of calculations performed with taking into account core relaxation and interaction between many resonances and many continua. The calculation shows that the resonance structure in the photoionization channels exists due to 4p 4 ( 1 D) 5s 2 D 5/2 6p 3/2 promoter state which also strongly perturbs the above Rydberg series.

Oscillatory behaviour of Rydberg state total cross sections in the collisions Ne+-He and He+-Ne

International Nuclear Information System (INIS)

Andresen, B.; Jensen, K.; Veje, E.

1976-01-01

The Ne + -He and He + -Ne collisions have been studied by means of optical spectrometry in the projectile energy range 10-150 keV. Very similar and regular oscillations in the Rydberg state total cross sections are found for HeI in both collisions and for singlet as well as triplet excitation. These oscillations are well described by the Rosenthal model. The HeI 4d sup(1,3)D states display two superimposed oscillations for center-of-mass collision energies above 6.4 keV. This is interpreted as the opening of a third exit channel, believed to be the HeI 4f sup(1,3)F. No, or very little structure is found in the Rydberg state total cross sections for HeII, NeI, NeII and NeIII levels. (Auth.)

Decay, excitation, and ionization of lithium Rydberg states by blackbody radiation

Science.gov (United States)

Ovsiannikov, V. D.; Glukhov, I. L.

2010-09-01

Details of interaction between the blackbody radiation and neutral lithium atoms were studied in the temperature ranges T = 100-2000 K. The rates of thermally induced decays, excitations and ionization were calculated for S-, P- and D-series of Rydberg states in the Fues' model potential approach. The quantitative regularities for the states of the maximal rates of blackbody-radiation-induced processes were determined. Approximation formulas were proposed for analytical representation of the depopulation rates.

Investigation of the Impact of Different Terms in the Second Order Hamiltonian on Excitation Energies of Valence and Rydberg States.

Science.gov (United States)

Tajti, Attila; Szalay, Péter G

2016-11-08

Describing electronically excited states of molecules accurately poses a challenging problem for theoretical methods. Popular second order techniques like Linear Response CC2 (CC2-LR), Partitioned Equation-of-Motion MBPT(2) (P-EOM-MBPT(2)), or Equation-of-Motion CCSD(2) (EOM-CCSD(2)) often produce results that are controversial and are ill-balanced with their accuracy on valence and Rydberg type states. In this study, we connect the theory of these methods and, to investigate the origin of their different behavior, establish a series of intermediate variants. The accuracy of these on excitation energies of singlet valence and Rydberg electronic states is benchmarked on a large sample against high-accuracy Linear Response CC3 references. The results reveal the role of individual terms of the second order similarity transformed Hamiltonian, and the reason for the bad performance of CC2-LR in the description of Rydberg states. We also clarify the importance of the T̂ 1 transformation employed in the CC2 procedure, which is found to be very small for vertical excitation energies.

Strongly perturbed Rydberg series originating from Kr II 4p45s ionic states

International Nuclear Information System (INIS)

Petrov, I.D.; Demekhin, P.V.; Lagutin, B.M.; Sukhorukov, V.L.; Kammer, S.; Mickat, S.; Schartner, K.-H.; Ehresmann, A.; Klumpp, S.; Werner, L.; Schmoranzer, H.

2004-01-01

Full text:Dispersed fluorescence excitation spectra for KrII fluorescence transitions to the 4p 4 5s 4 P 3/2 , 5/2 states were observed after excitation out of the KrI ground state with photons of energies between 28.4 eV and 28.7 eV and very narrow exciting-photon bandwidth of 1.7 meV. With this energy resolution it was possible to observe Rydberg series of doubly excited atomic states. The observed series were assigned to the states 4p 4 5s( 4 P 1/2 )np and 4p 4 5s( 2 P 3/2 )np ,based on calculations performed within theory taking into account interaction between many resonances and many continua. Calculated and measured cross sections are compared for the 4p - level (upper panel, ion yield) and for the 4p 4 5s 4 P 5/2 level (lower panel). An analysis of the computed photoionization (PI) cross sections shows that high - n members of Rydberg series are strongly perturbed by interaction with low - n ones of other series. In particular, the series shown are well pronounced because they borrow intensity from the low - n 4p 4 5s( 2 D 5/2 )6p 3/2 doublyexcited state. The above Rydberg series are predicted to be observable in photoelectron experiments, too. FIG. 1 shows, e.g., that members of the 4p 4 5s( 2 P 3/2 )np series starting from n 14 could also be observed in the 4p 4 5s 4P 1/2 observer channel at low photoelectron energies

Resonance-enhanced multiphoton ionization photoelectron spectroscopy of even-parity autoionizing Rydberg states of atomic sulphur

NARCIS (Netherlands)

Woutersen, S.; de Milan, J.B.; de Lange, C.A.; Buma, W.J.

1997-01-01

Several previously unobserved Rydberg states of the sulphur atom above the lowest ionization threshold are identified and assigned using (2 + 1) resonance-enhanced multiphoton-ionization photoelectron spectroscopy. All states were accessed by two-photon transitions from either the 3P ground or the

Lithium and rubidium extraction from zinnwaldite by alkali digestion process: Sintering mechanism and leaching kinetics

Czech Academy of Sciences Publication Activity Database

Vu, H.; Bernardi, J.; Jandová, J.; Vaculíková, Lenka; Goliáš, V.

2013-01-01

Roč. 123, č. 1 (2013), s. 9-17 ISSN 0301-7516 R&D Projects: GA MŠk ED2.1.00/03.0082 Institutional support: RVO:68145535 Keywords : zinnwaldite * lithium * rubidium * sintering mechanism * leaching kinetics Subject RIV: CB - Analytical Chemistry, Separation Impact factor: 1.461, year: 2013 http://www.sciencedirect.com/science/article/pii/S0301751613001087

ARC: An open-source library for calculating properties of alkali Rydberg atoms

Science.gov (United States)

Šibalić, N.; Pritchard, J. D.; Adams, C. S.; Weatherill, K. J.

2017-11-01

We present an object-oriented Python library for the computation of properties of highly-excited Rydberg states of alkali atoms. These include single-body effects such as dipole matrix elements, excited-state lifetimes (radiative and black-body limited) and Stark maps of atoms in external electric fields, as well as two-atom interaction potentials accounting for dipole and quadrupole coupling effects valid at both long and short range for arbitrary placement of the atomic dipoles. The package is cross-referenced to precise measurements of atomic energy levels and features extensive documentation to facilitate rapid upgrade or expansion by users. This library has direct application in the field of quantum information and quantum optics which exploit the strong Rydberg dipolar interactions for two-qubit gates, robust atom-light interfaces and simulating quantum many-body physics, as well as the field of metrology using Rydberg atoms as precise microwave electrometers. Program Files doi:http://dx.doi.org/10.17632/hm5n8w628c.1 Licensing provisions: BSD-3-Clause Programming language: Python 2.7 or 3.5, with C extension External Routines: NumPy [1], SciPy [1], Matplotlib [2] Nature of problem: Calculating atomic properties of alkali atoms including lifetimes, energies, Stark shifts and dipole-dipole interaction strengths using matrix elements evaluated from radial wavefunctions. Solution method: Numerical integration of radial Schrödinger equation to obtain atomic wavefunctions, which are then used to evaluate dipole matrix elements. Properties are calculated using second order perturbation theory or exact diagonalisation of the interaction Hamiltonian, yielding results valid even at large external fields or small interatomic separation. Restrictions: External electric field fixed to be parallel to quantisation axis. Supplementary material: Detailed documentation (.html), and Jupyter notebook with examples and benchmarking runs (.html and .ipynb). [1] T.E. Oliphant

Crystal structure of rubidium methyl-diazo-tate.

Science.gov (United States)

Grassl, Tobias; Korber, Nikolaus

2017-02-01

The title compound, Rb + ·H 3 CN 2 O - , has been crystallized in liquid ammonia as a reaction product of the reductive ammonolysis of the natural compound streptozocin. Elemental rubidium was used as reduction agent as it is soluble in liquid ammonia, forming a blue solution. Reductive bond cleavage in biogenic materials under kinetically controlled conditions offers a new approach to gain access to sustainably produced raw materials. The anion is nearly planar [dihedral angle O-N-N-C = -0.4 (2)°]. The Rb + cation has a coordination number of seven, and coordinates to five anions. One anion is bound via both its N atoms, one by both O and N, two anions are bound by only their O atoms, and the last is bound via the N atom adjacent to the methyl group. The diazo-tate anions are bridged by cations and do not exhibit any direct contacts with each other. The cations form corrugated layers that propagate in the (-101) plane.

Observation of the Stark effect in υ+ = 0 Rydberg states of NO: a comparison between predissociating and bound states

International Nuclear Information System (INIS)

Jones, N J A; Minns, R S; Patel, R; Fielding, H H

2008-01-01

The Stark spectra of Rydberg states of NO below the υ + = 0 ionization limit, with principal quantum numbers n = 25-30, have been investigated in the presence of dc electric fields in the range 0-150 V cm -1 . The Stark states were accessed by two-colour, double-resonance excitation via the υ' = 0, N' = 0 rovibrational state of the A 2 Σ + state. The N( 2 D) atoms produced by predissociation were measured by (2 + 1) resonance-enhanced multiphoton ionization, and compared with pulsed-field ionization spectra of the bound Rydberg state population (Patel et al 2007 J. Phys. B: At. Mol. Opt. Phys. 40 1369)

Ionization of xenon Rydberg atoms at Si(1 0 0) surfaces

Energy Technology Data Exchange (ETDEWEB)

Dunham, H.R. [Department of Physics and Astronomy, Rice University MS-61, 6100 Main Street, Houston, TX 77005-1892 (United States); Wethekam, S. [Institut fuer Physik der Humboldt-Universitaet zu Berlin, Newtonstra. 15, D-12489, Berlin (Germany); Lancaster, J.C. [Department of Physics and Astronomy, Rice University MS-61, 6100 Main Street, Houston, TX 77005-1892 (United States); Dunning, F.B. [Department of Physics and Astronomy, Rice University MS-61, 6100 Main Street, Houston, TX 77005-1892 (United States)]. E-mail: fbd@rice.edu

2007-03-15

The ionization of xenon Rydberg atoms excited to the lowest states in the n = 17 and n = 20 Stark manifolds at Si(1 0 0) surfaces is investigated. It is shown that, under appropriate conditions, a sizable fraction of the incident atoms can be detected as ions. Although the onset in the ion signal is perturbed by stray fields present at the surface, the data are consistent with ionization rates similar to those measured earlier at metal surfaces.

Coherence effects in three- and four-level laser-cooled rubidium systems

International Nuclear Information System (INIS)

De Echaniz, Sebastian R.

2002-01-01

This thesis presents developmental work on the existing magneto-optical trap (MOT) system and novel studies of coherence effects. The developmental work was carried out on the experimental apparatus used previously in this laboratory in order to perform experiments to study coherence effects in three- and four-level rubidium systems in the MOT. This developmental work includes the upgrading and installation of new laser systems, the improvement of the MOT, the installation of data acquisition hardware and software, and the commissioning of a new 'second generation' MOT. As part of our studies of coherence effects, we present a wide-ranging theoretical and experimental study of non-adiabatic transient phenomena in a Λ system which exhibits electromagnetically induced transparency when a strong coupling field is rapidly switched on or off using a Pockels cell. The theoretical treatment uses a Laplace transform approach as well as standard numerical methods to solve the time-dependent density matrix equation. The results show clear Rabi oscillations and transient gain without population inversion of a weak probe in parameter regions not previously studied, and provide insight into the transition dynamics between bare a dressed states. Experimental studies of a doubly driven V system are also reported, together with a theoretical dressed-state analysis of such systems. The expected three-peak spectrum is explored for various coupling field strengths and detunings. In all this work we have found good agreement between the theory and the experimental spectra once light shifts and uncoupled absorption in the rubidium system are taken into account. (author)

Interaction of Rydberg atoms in circular states with the alkaline-earth Ca(4s{sup 2}) and Sr(5s{sup 2}) atoms

Energy Technology Data Exchange (ETDEWEB)

Mironchuk, E. S.; Narits, A. A.; Lebedev, V. S., E-mail: vlebedev@sci.lebedev.ru [Russian Academy of Sciences, Lebedev Physical Institute (Russian Federation)

2015-11-15

The resonant mechanism of interaction of alkaline-earth atoms having a low electron affinity to Rydberg atoms in circular (l = vertical bar m vertical bar = n–1) and near-circular states has been studied. To describe the dynamics of resonant processes accompanied by nonadiabatic transitions between ionic and Rydberg covalent terms of a quasimolecule, an approach based on the integration of coupled equations for the probability amplitudes has been developed taking into account the possibility of the decay of an anion in the Coulomb field of the positive ionic core of a highly excited atom. The approach involves the specific features of the problem associated with the structure of the wavefunction of a Rydberg electron in states with high orbital angular momenta l ∼ n–1. This approach provides a much more accurate description of the dynamics of electronic transitions at collisions between atoms than that within the modified semiclassical Landau–Zener model. In addition, this approach makes it possible to effectively take into account many channels of the problem. The cross sections for resonant quenching of Rydberg states of the Li(nlm) atom with given principal n, orbital l = n–1, and magnetic m quantum numbers at thermal collisions with the Ca(4s{sup 2}) and Sr(5s{sup 2}) atoms have been calculated. The dependences of the results on n, m, and angle α between the relative velocity of the atoms and the normal to the plane of the orbit of the Rydberg electron have been obtained. The influence of orientational effects on the efficiency of the collisional destruction of circular and near-circular states has been studied. The results indicate a higher stability of such states to their perturbations by neutral particles as compared to usually studied nl states with low values of l (l ≪ n)

Properties of Fr-like Th^3+ from microwave spectroscopy of high-L Rydberg states of Th^2+

Science.gov (United States)

Keele, Julie; Smith, Chris; Woods, Shannon; Lundeen, Stephen; Fehrenbach, Charles

2012-06-01

Spectroscopy of high-L n= 28 Rydberg levels of Th^2+ was recently reported using the optical RESIS method [1]. Because the ground state of Fr-like Th^3+ is a ^2F5/2 level, each (n,L) Rydberg level of Th^2+ is split into six eigenstates whose relative positions are determined by long-range e-Th^3+ interactions. Measurements of those positions can be used to determine the Th^3+ properties that control those interactions, such as polarizabilities and permanent moments. We report a much improved study of n=28 levels with 9 Hanni, Shannon L. Woods, S.R. Lundeen, and C.W. Fehrenbach, Phys. Rev. A 83, 062501 (2011)[0pt] [2] U.I. Safronova, W.R. Johnson, and M.S. Safronova, Phys. Rev. A 74, 042511 (2006)

Photoionization microscopy of Rydberg hydrogen atom in a non-uniform electrical field

International Nuclear Information System (INIS)

Cheng Shao-Hao; Wang De-Hua; Chen Zhao-Hang; Chen Qiang

2016-01-01

In this paper, we investigate the photoionization microscopy of the Rydberg hydrogen atom in a gradient electric field for the first time. The observed oscillatory patterns in the photoionization microscopy are explained within the framework of the semiclassical theory, which can be considered as a manifestation of interference between various electron trajectories arriving at a given point on the detector plane. In contrast with the photoionization microscopy in the uniform electric field, the trajectories of the ionized electron in the gradient electric field will become chaotic. An infinite set of different electron trajectories can arrive at a given point on the detector plane, which makes the interference pattern of the electron probability density distribution extremely complicated. Our calculation results suggest that the oscillatory pattern in the electron probability density distribution depends sensitively on the electric field gradient, the scaled energy and the position of the detector plane. Through our research, we predict that the interference pattern in the electron probability density distribution can be observed in an actual photoionization microscopy experiment once the external electric field strength and the position of the electron detector plane are reasonable. This study provides some references for the future experimental research on the photoionization microscopy of the Rydberg atom in the non-uniform external fields. (paper)

Self-excitation of Rydberg atoms at a metal surface

DEFF Research Database (Denmark)

Bordo, Vladimir

2017-01-01

The novel effect of self-excitation of an atomic beam propagating above a metal surface is predicted and a theory is developed. Its underlying mechanism is positive feedback provided by the reflective surface for the atomic polarization. Under certain conditions the atomic beam flying in the near...... field of the metal surface acts as an active device that supports sustained atomic dipole oscillations, which generate, in their turn, an electromagnetic field. This phenomenon does not exploit stimulated emission and therefore does not require population inversion in atoms. An experiment with Rydberg...... atoms in which this effect should be most pronounced is proposed and the necessary estimates are given....

Nonspreading Wave Packets for Rydberg Electrons in Rotating Molecules with Electric Dipole Moments

International Nuclear Information System (INIS)

Bialynicki-Birula, I.; Bialynicka-Birula, Z.

1996-01-01

Nonspreading wave packets for Rydberg electrons are predicted in rotating molecules with electric dipole moments. We have named them the Trojan wave packets since their stability is due to the same mechanism that governs the motion of the Trojan asteroids in the Sun-Jupiter system. Unlike all previously predicted Trojan wave packets in atoms, molecular Trojan states do not require external fields for their existence

Ramsey interferometry of Rydberg ensembles inside microwave cavities

Science.gov (United States)

Sommer, Christian; Genes, Claudiu

2018-06-01

We study ensembles of Rydberg atoms in a confined electromagnetic environment such as is provided by a microwave cavity. The competition between standard free space Ising type and cavity-mediated interactions leads to the emergence of different regimes where the particle‑particle couplings range from the typical van der Waals r ‑6 behavior to r ‑3 and to r-independence. We apply a Ramsey spectroscopic technique to map the two-body interactions into a characteristic signal such as intensity and contrast decay curves. As opposed to previous treatments requiring high-densities for considerable contrast and phase decay (Takei et al 2016 Nat. Comms. 7 13449; Sommer et al 2016 Phys. Rev. A 94 053607), the cavity scenario can exhibit similar behavior at much lower densities.

Rubidium in the food chain

Energy Technology Data Exchange (ETDEWEB)

Anke, M. [Inst. of Nutrition and Environment, Friedrich Schiller Univ., Jena (Germany); Angelow, L. [Inst. of Nutrition and Environment, Friedrich Schiller Univ., Jena (Germany)

1995-05-01

In spite of its abundant occurrence in the earth`s crust (310 mg Rb/kg) and its composition of a stable (72.2%) and a radioactive (27.8%) isotope, rubidium (Rb) belongs to the forgotten ultratrace elements. The interest in this ultratrace element grew considerably after Rb deficiency experiments with goats had shown that their growth was depressed, that > 80% of them aborted their kids. The geological origin of the site takes significant effect on the Rb content of the flora. Granite and gneiss weathering soils produce the by far Rb-richest plant populations, and drinking water. The water of the gneiss sites contained 18 {mu}g Rb/l, that of diluvial sands 3 {mu}g/l. Herbivores store most Rb whereas carnivores and omnivores accumulate significantly less Rb. The analysis of 137 foodstuffs and beverages in 15-fold repetition showed that the starch- and sugar-rich cereals, pasta, bread and confectionary are poor in Rb (1 mg/kg dry mater (DM)). Fruit and vegetables accumulate between 5 and > 60 mg Rb/kg (asparagus). Boiling drastically reduces the Rb content of vegetables. Animal foodstuffs are relatively poor in Rb. Poultry meat as well as freshwater fish are relatively rich in Rb. Coffee (40 mg/kg DM) and black tea (100 mg Rb/kg DM) store much Rb, 85% of which pass into the beverage. (orig.)

Observation of Rydberg transitions from the inner valence shell of ethane

International Nuclear Information System (INIS)

Dillon, M.A.; Tanaka, H.; Spence, D.

1987-01-01

The electron impact spectrum of ethane has been examined in a region that includes ionization out of the inner valence shell. One diffuse structure and a progression of ten vibrational bands have been found in a 4 eV range below and to some degree overlapping the 2 A 2 /sub u/ ion threshold. Evidence indicates that the observed transitions belong to the symmetry forbidden Rydberg series (2a 2 /sub u/) 2 →(2a 2 /sub u/, npσ or npπ)

Excited states of ethylene interpreted in terms of perturbed Rydberg series

International Nuclear Information System (INIS)

Yamamoto, Shigeyoshi; Tatewaki, Hiroshi

2003-01-01

We have investigated the excited states of the ethylene molecule by the multireference configuration interaction (MRCI) method. In particular, the nature of the V state (1 1 B 1u π→π*) was interpreted in terms of perturbed Rydberg series. To clarify the role of the perturbers, we use pseudo-restricted Hartree-Fock natural orbitals (PRHFNO), which would be the most suitable molecular orbital set to describe Rydberg series. It is well known that the expectation value of x 2 for the V state is reduced from 44a 0 2 (RHF) to around 17a 0 2 by considering electron correlation effects, where x is the direction out of the molecular plane. In the present study, a reasonable 2 > value was obtained from small multireference configuration interaction with single excitations (MRCIS), where the π→π* configurations and a few perturbers were assigned as the reference configurations. The major perturbers were found to be five configurations represented by 3a g → 3b 1u , 1b 3g → 3b 2u , 2b 1u → 4a g , 2a g → 3b 1u , and 1b 2u → 2b 3g with respect to the ground state configuration. The V state can therefore be described as a scattering process of the π→π* state by these perturbers. Other low-lying excited states are also investigated by the MRCI method

The importance of Rydberg orbitals in dissociative ionization of small hydrocarbon molecules in intense laser fields.

Science.gov (United States)

Jochim, Bethany; Siemering, R; Zohrabi, M; Voznyuk, O; Mahowald, J B; Schmitz, D G; Betsch, K J; Berry, Ben; Severt, T; Kling, Nora G; Burwitz, T G; Carnes, K D; Kling, M F; Ben-Itzhak, I; Wells, E; de Vivie-Riedle, R

2017-06-30

Much of our intuition about strong-field processes is built upon studies of diatomic molecules, which typically have electronic states that are relatively well separated in energy. In polyatomic molecules, however, the electronic states are closer together, leading to more complex interactions. A combined experimental and theoretical investigation of strong-field ionization followed by hydrogen elimination in the hydrocarbon series C 2 D 2 , C 2 D 4 and C 2 D 6 reveals that the photofragment angular distributions can only be understood when the field-dressed orbitals rather than the field-free orbitals are considered. Our measured angular distributions and intensity dependence show that these field-dressed orbitals can have strong Rydberg character for certain orientations of the molecule relative to the laser polarization and that they may contribute significantly to the hydrogen elimination dissociative ionization yield. These findings suggest that Rydberg contributions to field-dressed orbitals should be routinely considered when studying polyatomic molecules in intense laser fields.

A thermodynamic assessment of the behavior of cesium and rubidium in reactor fuel elements

International Nuclear Information System (INIS)

Kohli, R.

1981-01-01

A comprehensive thermodynamic model is developed to assess the reaction and transport behavior of fission products in LWR fuel elements. The emphasis is on the chemistry of cesium and rubidium and their reactions with the fuel, other fission products, and the zircaloy cladding. Equilibrium thermodynamic calculations have been performed on the most plausible reactions to predict the chemical state of the fission products. The relevance of the predictions to pellet-clad interaction failures is discussed in detail. (orig.)

Adsorption of Cesium, Strontium, and Rubidium radionuclides in the Mag-molecular process: The influence of important factors

Directory of Open Access Journals (Sweden)

Fatemeh Tangestani

2017-09-01

Full Text Available In this study, the adsorption of cesium, strontium, and rubidium radionuclides by ferritin magmolecules in a batch system was investigated under different experimental conditions. The experiments were conducted in a pilot plant that involved the contactor unit and the magnetic separator unit. The impact of the pollutant concentrations, adsorbent concentration, and pH on the efficiency of the process were investigated thoroughly. The maximum recovery of radionuclides in the studied domain were 57.05%, 85.42% and 71.82% for Cs+, Sr2+ and Rb+ ,respectively, in which the pollutant concentration was 363.63 mg/l, the adsorbent concentration was 0.011 g/l, and the pH was 7.5. The results showed that the ferritin adsorbent in the magmolecular process manifested a higher efficiency in adsorbing the bivalent ions of strontium compared to the univalent ions of cesium and rubidium. Furthermore, the results were statistically analyzed and the model and residual plots of each radionuclide were presented. The results also signified  relationships between the independent variables and recovery.

Noninvasive quantification of regional myocardial perfusion with rubidium-82 and positron emission tomography. Exploration of a mathematical model

International Nuclear Information System (INIS)

Herrero, P.; Markham, J.; Shelton, M.E.; Weinheimer, C.J.; Bergmann, S.R.

1990-01-01

Positron emission tomography (PET) centers without cyclotrons use generator-produced rubidium-82 (82Rb) for assessment of myocardial perfusion. The aim of the present study was to determine whether myocardial blood flow could be assessed quantitatively with 82Rb and PET. Because the myocardial extraction fraction of 82Rb varies inversely and nonlinearly with flow and cannot be measured conveniently with PET, we used an experimentally derived mathematical function defining the relation between single-pass extraction fraction of 82Rb and flow to obviate the necessity of measuring the extraction fraction directly. Myocardial blood flow in absolute terms (ml/g/min) was estimated from dynamic PET scans after intravenous administration of 82Rb in intact dogs and compared with flows measured with radiolabeled microspheres. In 36 comparisons in 13 dogs studied at rest, or after coronary occlusion, reperfusion, or after coronary hyperemia induced with intravenous dipyridamole, over the flow range from 0.2 to 2.0 ml/g/min, estimates of perfusion with rubidium correlated well with flows measured concomitantly with microspheres, although there was a slight underestimation of flow with rubidium (flow by 82Rb = 0.92 x flow by microspheres-0.021, r = 0.83). In general, estimates of flow in ischemic regions were less reliable than estimates for regions with normal flow. Thus, although the relation between myocardial extraction and retention of 82Rb and flow can vary under a variety of physiological and pathophysiological conditions, this study demonstrates the ability to obtain quantitative estimates of myocardial blood flow with 82Rb and PET under carefully defined conditions without measuring the extraction fraction directly

The Rydberg constant and proton size from atomic hydrogen

Science.gov (United States)

Beyer, Axel; Maisenbacher, Lothar; Matveev, Arthur; Pohl, Randolf; Khabarova, Ksenia; Grinin, Alexey; Lamour, Tobias; Yost, Dylan C.; Hänsch, Theodor W.; Kolachevsky, Nikolai; Udem, Thomas

2017-10-01

At the core of the “proton radius puzzle” is a four-standard deviation discrepancy between the proton root-mean-square charge radii (rp) determined from the regular hydrogen (H) and the muonic hydrogen (µp) atoms. Using a cryogenic beam of H atoms, we measured the 2S-4P transition frequency in H, yielding the values of the Rydberg constant R∞ = 10973731.568076(96) per meterand rp = 0.8335(95) femtometer. Our rp value is 3.3 combined standard deviations smaller than the previous H world data, but in good agreement with the µp value. We motivate an asymmetric fit function, which eliminates line shifts from quantum interference of neighboring atomic resonances.

Microwave spectroscopy of high-L Rydberg states of nickel

Science.gov (United States)

Lindsay, Mark D.; Keele, Julie A.; Woods, Shannon L.; Lundeen, Stephen R.

2010-03-01

High-L non-penetrating Rydberg levels of nickel display a fine structure pattern consisting of six levels for each value of L. This pattern was studied recently with the optical RESIS technique, determining initial values of the quadrupole moment and polarizabilities of the ^2D5/2 ground state of Ni^+ [1]. Measurements are now in progress using the microwave RESIS technique [2], which promises much more precise measurements of the fine structure and of the related core properties, including the permanent hexadecapole moment.[4pt] [1] Julie A. Keele, et. al., to be published, Phys. Rev. A[0pt] [2] M.E. Hanni, et. al., Phys. Rev. A 78, 062510 (2008)

Atoms, cavities and ''Schroedinger's cats''. The monsters and wonders of quantum mechanics

International Nuclear Information System (INIS)

Raimond, J.M.

1997-01-01

The decoherence effect appears at the border between quantum world and macroscopic reality when the superposition of quantum states collapses into one particular state. This article deals with an experiment made to study for the first time the decoherence phenomenon. Circular Rydberg atoms of rubidium and superconducting cavity are the tools used to seize the very moment when the quantum superposition vanishes. This experimental proof of decoherence allows to perceive the limitations of the applications of quantum physics to fields such as quantum computing. This kind of experiment could be used to test other properties of quantum systems. (A.C.)

Rubidium 2,4,6-trioxo-1,3-diazinan-5-ide–1,3-diazinane-2,4,6-trione–water (1/1/1

Directory of Open Access Journals (Sweden)

Marlena Gryl

2011-05-01

Full Text Available The asymmetric unit of the title compound, Rb+·C4H3N2O3−·C4H4N2O3·H2O, consists of one rubidium cation, a barbituric acid molecule, a barbiturate anion and one water molecule. The rubidium ion has seven close-contact interactions with O atoms, with Rb...O distances ranging from 2.8594 (16 to 3.2641 (14 Å. These seven O atoms together with an eighth O atom at 3.492 (2 Å away from Rb form a distorted polyhedron with shape intermediate between an antiprism and a dodecahedron. The Rb+ ions connect layers built of organic components and water molecules linked via N—H...O and O—H...O hydrogen bonds.

Formation of cold molecules through the photo-association of cold atoms of Cesium. Existence of long range forces between between cold excited atoms of Cesium; Formation de molecules froides par photoassociation d'atomes froids de cesium. Mise en evidence de forces a longue portee entre atomes froids excites de cesium

Energy Technology Data Exchange (ETDEWEB)

Comparat, D

1999-09-01

This thesis deals with the experimental study and the theoretical interpretation of the processes involved in photo-association and the formation of cold caesium molecules. It also presents a study of the dipolar forces between a pair of cold excited caesium atoms. We present here the first photo-association experiment on cold caesium atoms: two cold atoms absorb a photon to form an excited electronically excited molecules in a rotation-vibration level. The first production of cold molecules which was realised experimentally, after the spontaneous deexcitation of the photo-associated molecules, is described, stressing the role of the potential well of the molecular states O{sub g}{sup -}(6s+6p{sub 3/2}) or 1{sub u} (6s+6p{sub 3/2}) of caesium. The detection of the formed caesium molecules is based on a two-photons resonant ionisation that creates Cs{sub 2}{sup +} ions, afterwards selectively detected. Temperatures around 20-200 {mu}K have been measured. The photo-associative spectroscopy is described on the theoretical point of view: a detailed theoretical study allows to calculate precisely the asymptotic parts of the potential curves. On the experimental point of view, we present the spectroscopy of the extern potential well of the caesium state O{sub g}{sup -}(6s+6p{sub 3/2}) and the construction of an effective potential curve of the RKR type. A unified theory of photo-association in weak field, considered as a collision assisted by laser, is developed. The cold atoms experiments allow to study and control the collision between two atoms whose mutual interaction is of the dipole-dipole type. Two different physical systems are studied: a sample of Rydberg atoms, and the photo-association process which is a laser-assisted collision. A modification of the motion of one pair of atoms makes it possible to control the bipolar forces and to choose the atoms relative speeds. (author)

A new method for detecting the contribution of high Rydberg states to electron-ion recombination

International Nuclear Information System (INIS)

Orban, I; Boehm, S; Fogle, M; Paal, A; Schuch, R

2007-01-01

A position sensitive detector for measuring field ionized electrons in the fringe field of a dipole magnet is presented. The detector provides a means to study, in a state selective fashion, recombination into high Rydberg states and offers a new method to investigate recombination enhancement effects. Several experimental considerations and possibilities are discussed in the text

Story of rubidium-82 and advantages for myocardial perfusion PET imaging

Directory of Open Access Journals (Sweden)

Jean-Francois eChatal

2015-09-01

Full Text Available Rubidium-82 has a long story, starting in 1954. After preclinical studies in dogs showing that myocardial uptake of this radionuclide was directly proportional to myocardial blood flow, clinical studies were performed in the 80s leading to an approval in the USA in 1989. From that time thousands of patients have been tested and their results have been reported in 3 meta-analyses. Pooled patient-based sensitivity and specificity were respectively 0.91 and 0.90. By comparison with 99mTc-SPECT, 82Rb-PET had a much better diagnostic accuracy, especially in obese patients with BMI (Body Mass Index ≥30 kg/m2 (85% versus 67% with SPECT and in women with large breasts. A great advantage of 82Rb-PET is its capacity to accurately quantify myocardial blood flow. Quite importantly it has been recently shown that coronary flow reserve is associated with adverse cardiovascular events independently of luminal angiographic severity. Moreover coronary flow reserve is a functional parameter particularly useful in the estimate of microvascular dysfunction such as in diabetes mellitus. Due to the very short half-life of rubidium-82, the effective dose calculated for a rest/stress test is roughly equivalent to the annual natural exposure and even less when stress-only is performed with a low activity compatible with a good image quality with the last generation 3D PET scanners.There is still some debate on the relative advantages of 82Rb-PET with regard to 99mTc-SPECT. For the last ten years, great technological advances substantially improved performances of SPECT with its accuracy getting closer to this of 82Rb/PET. Currently the main advantages of PET are its capacity to accurately quantify myocardial blood flow and to deliver a low radiation exposure.

Exciton induced directed motion of unconstrained atoms in an ultracold gas

Science.gov (United States)

Leonhardt, K.; Wüster, S.; Rost, J. M.

2017-03-01

We demonstrate that through localised Rydberg excitation in a three-dimensional cold atom cloud atomic motion can be rendered directed and nearly confined to a plane, without spatial constraints for the motion of individual atoms. This enables creation and observation of non-adiabatic electronic Rydberg dynamics in atoms accelerated by dipole-dipole interactions under natural conditions. Using the full l = 0, 1 m=0,+/- 1 angular momentum state space, our simulations show that conical intersection crossings are clearly evident, both in atomic position information and excited state spectra of the Rydberg system. Hence, flexible Rydberg aggregates suggest themselves for probing quantum chemical effects in experiments on length scales much inflated as compared to a standard molecular situation.

Pump-probe study of the formation of rubidium molecules by ultrafast photoassociation of ultracold atoms

Science.gov (United States)

McCabe, David J.; England, Duncan G.; Martay, Hugo E. L.; Friedman, Melissa E.; Petrovic, Jovana; Dimova, Emiliya; Chatel, Béatrice; Walmsley, Ian A.

2009-09-01

An experimental pump-probe study of the photoassociative creation of translationally ultracold rubidium molecules is presented together with numerical simulations of the process. The formation of loosely bound excited-state dimers is observed as a first step toward a fully coherent pump-dump approach to the stabilization of Rb2 into its lowest ground vibrational states. The population that contributes to the pump-probe process is characterized and found to be distinct from a background population of preassociated molecules.

Proposal for making a beam of antihydrogen by two charge exchange events

International Nuclear Information System (INIS)

Robicheaux, F

2010-01-01

We have performed calculations of two successive charge transfers in a geometry that could generate a beam of antihydrogen atoms (H-bar) or reliably produce cold H-bar without having to reach extremely cold plasma temperatures. The basic idea is similar to that proposed by Hessels et al (1998 Phys. Rev. A 57 1668) except that the order of the charge transfers is reversed. A beam of highly-excited (Rydberg) Cs atoms passes through an antiproton (p-bar) plasma where a charge transfer can take place; the result is an exotic Rydberg atom (Cs + ion and a bound p-bar) which has approximately the original velocity of the Cs atom since the Cs + mass is much greater than that of the p-bar. This exotic Rydberg atom travels into a positron plasma where a second charge exchange gives antihydrogen (H-bar). The velocity distribution of the resulting H-bar is directly related to the original velocity of the Rydberg Cs atom. The binding energy of the H-bar is roughly that of the original Cs Rydberg atom; thus, the starting state of the H-bar can be controlled by choosing the initial state of the Cs atom. Because the p-barCs + binding energy can be controlled in the charge transfer, this first step, by itself, could be of interest to the exotic atom community.

Dissociative electron attachment to vibrationally excited H2 molecules involving the 2Σg+ resonant Rydberg electronic state

International Nuclear Information System (INIS)

Celiberto, R.; Janev, R.K.; Wadehra, J.M.; Tennyson, J.

2012-01-01

Graphical abstract: Dissociative electron attachment cross sections as a function of the incident electron energy and for the initial vibration levels v i = 0–5, 10 of the H 2 molecule. Highlights: ► We calculated electron–hydrogen dissociative attachment cross sections and rates coefficients. ► Collision processes occurring through a resonant Rydberg state are considered. ► Cross sections and rates were obtained for vibrationally excited hydrogen molecules. ► The cross sections exhibit pronounced oscillatory structures. ► A comparison with the process involving the electron–hydrogen resonant ground state is discussed. - Abstract: Dissociative electron attachment cross sections (DEA) on vibrationally excited H 2 molecule taking place via the 2 Σ g + Rydberg-excited resonant state are studied using the local complex potential (LCP) model for resonant collisions. The cross sections are calculated for all initial vibrational levels (v i = 0–14) of the neutral molecule. In contrast to the previously noted dramatic increase in the DEA cross sections with increasing v i , when the process proceeds via the X 2 Σ u + shape resonance of H 2 , for the 2 Σ g + Rydberg resonance the cross sections increase only gradually up to v i = 3 and then decrease. Moreover, the cross sections for v i ⩾ 6 exhibit pronounced oscillatory structures. A discussion of the origin of the observed behavior of calculated cross sections is given. The DEA rate coefficients for all v i levels are also calculated in the 0.5–1000 eV temperature range.

Dynamics of solvation and desolvation of rubidium attached to He nanodroplets

International Nuclear Information System (INIS)

Vangerow, J. von; John, O.; Stienkemeier, F.; Mudrich, M.

2015-01-01

The real-time dynamics of photoexcited and photoionized rubidium (Rb) atoms attached to helium (He) nanodroplets is studied by femtosecond pump-probe mass spectrometry. While excited Rb atoms in the perturbed 6p-state (Rb * ) desorb off the He droplets, Rb + photoions tend to sink into the droplet interior when created near the droplet surface. The transition from Rb + solvation to full Rb * desorption is found to occur at a delay time τ ∼ 600 fs for Rb * in the 6pΣ-state and τ ∼ 1200 fs for the 6pΠ-state. Rb + He ions are found to be created by directly exciting bound Rb * He exciplex states as well as by populating bound Rb + He-states in a photoassociative ionization process

Dynamics of solvation and desolvation of rubidium attached to He nanodroplets

Science.gov (United States)

von Vangerow, J.; John, O.; Stienkemeier, F.; Mudrich, M.

2015-07-01

The real-time dynamics of photoexcited and photoionized rubidium (Rb) atoms attached to helium (He) nanodroplets is studied by femtosecond pump-probe mass spectrometry. While excited Rb atoms in the perturbed 6p-state (Rb*) desorb off the He droplets, Rb+ photoions tend to sink into the droplet interior when created near the droplet surface. The transition from Rb+ solvation to full Rb* desorption is found to occur at a delay time τ ˜ 600 fs for Rb* in the 6pΣ-state and τ ˜ 1200 fs for the 6pΠ-state. Rb+He ions are found to be created by directly exciting bound Rb*He exciplex states as well as by populating bound Rb+He-states in a photoassociative ionization process.

Dynamic polarizabilities and Rydberg states of the argon isoelectronic sequence

International Nuclear Information System (INIS)

Ghosh, T.K.; Das, A.K.; Castro, M.; Canuto, S.; Mukherjee, P.K.

1993-01-01

Dynamic dipole polarizabilities α d (ω) have been calculated within and beyond the normal-dispersion region for the isoelectronic members of argon up to Mn 7+ using time-dependent coupled Hartree-Fock theory. Excitation energies, oscillator strengths, and quantum-defect values have been estimated for the dipole-allowed transitions 3p 6 1 Se→3p 5 ( 2 P)ns 1 Po (n=4,...,7) and 3p 6 1 Se→3p 5 ( 2 P)nd 1 Po (n=3,...,7). Analytic representations of the singly excited Rydberg orbitals have been obtained. The results compare favorably with the existing theoretical and experimental data. The oscillator strengths show an interesting trend of variation along the isoelectronic sequence

Radiation Pressure in a Rubidium Optical Lattice: An Atomic Analog to the Photorefractive Effect

International Nuclear Information System (INIS)

Guibal, S.; Mennerat-Robilliard, C.; Larousserie, D.; Triche, C.; Courtois, J.; Grynberg, G.

1997-01-01

Probe gain in a rubidium optical lattice is observed when the probe and lattice beams have identical frequencies. This effect is shown to arise from the radiation pressure that shifts the atomic density distribution with respect to the optical potential. This effect is compared with two-beam coupling in photorefractive materials. The experimental results obtained by changing the parameters of the optical lattice (intensity, detuning, periodicity) are in reasonable agreement with numerical simulations based on the model case of a 1/2→3/2 atomic transition. copyright 1997 The American Physical Society

Radiative transitions from Rydberg states of lithium atoms in a blackbody radiation environment

Science.gov (United States)

Glukhov, I. L.; Ovsiannikov, V. D.

2012-05-01

The radiative widths induced by blackbody radiation (BBR) were investigated for Rydberg states with principal quantum number up to n = 1000 in S-, P- and D-series of the neutral lithium atom at temperatures T = 100-3000 K. The rates of BBR-induced decays and excitations were compared with the rates of spontaneous decays. Simple analytical approximations are proposed for accurate estimations of the ratio of thermally induced decay (excitation) rates to spontaneous decay rates in wide ranges of states and temperatures.

The population transfer of high excited states of Rydberg lithium atoms in a microwave field

International Nuclear Information System (INIS)

Jiang Lijuan; Zhang Xianzhou; Ma Huanqiang; Jia Guangrui; Zhang Yonghui; Xia Lihua

2012-01-01

Using the time-dependent multilevel approach (TDMA), the properties of high excited Rydberg lithium atom have been obtained in the microwave field. The population transfer of lithium atom are studied on numerical calculation, quantum states are controlled and manipulated by microwave field. It shows that the population can be completely transferred to the target state by changing the chirped rate and field amplitude. (authors)

Inner-shell spectroscopy and exchange interaction of Rydberg electrons bound by singly and doubly charged Kr and Xe atoms in small clusters

International Nuclear Information System (INIS)

Nagasaka, Masanari; Hatsui, Takaki; Setoyama, Hiroyuki; Ruehl, Eckart; Kosugi, Nobuhiro

2011-01-01

Surface-site resolved Kr 3d 5/2 -1 5p and 3d 5/2 -1 6p and Xe 4d 5/2 -1 6p and 4d 5/2 -1 7p Rydberg excited states in small van der Waals Kr and Xe clusters with a mean size of = 15 are investigated by X-ray absorption spectroscopy. Furthermore, surface-site resolved Kr 4s -2 5p, 4s -2 6p, and 4s -1 4p -1 5p shakeup-like Rydberg states in small Kr clusters are investigated by resonant Auger electron spectroscopy. The exchange interaction of the Rydberg electron with the surrounding atoms and the induced polarization of the surrounding atoms in the singly and doubly ionized atoms are deduced from the experimental spectra to analyze different surface-site contributions in small clusters, assuming that the corner, edge, face, and bulk sites have 3, 5-6, 8, and 12 nearest neighbor atoms. These energies are almost proportional to the number of the nearest neighbor atoms. The present analysis indicates that small Kr and Xe clusters with = 15 have an average or mixture structure between the fcc-like cubic and icosahedron-like spherical structures.

Demonstration of bicolor slow-light channelization in rubidium vapor

International Nuclear Information System (INIS)

Bashkansky, Mark; Fatemi, Fredrik K.; Reintjes, John; Dutton, Zachary; Steiner, Michael

2007-01-01

We experimentally demonstrate a proof-of-principle of a previously proposed 'channelization' architecture for wideband slow-light propagation in atomic vapors using electromagnetically induced transparency (EIT). We use two optical frequencies to generate a sine wave signal which is delayed in rubidium vapor. The optical frequencies were tuned near the EIT resonances of two Zeeman sublevels, which are shifted from each other well beyond the EIT linewidth by a uniform magnetic field. We varied the Zeeman shift between these two levels (relative to the optical frequency splitting) and measured the delay versus Zeeman shift. Significant delays were observed and were in agreement with a theoretical model treating each Zeeman sublevel as part of an independent three-level system. We achieved delay of a signal with a bandwidth 16 times the EIT linewidth and confirmed our earlier theoretical models that delay occurs only when the optical spectral separation slightly exceeds the Zeeman splitting

The structure factor and the pair potential of liquid rubidium at temperatures between 450 K and 1,400 K

International Nuclear Information System (INIS)

Block de Priego, R.A.

1977-11-01

The structure factor S(Q) of liquid rubidium has been measured for temperatures between 450 K and 1400 K and pressures up to 200 atm. The corresponding densities varied between 1.42 and 0.98 g cm -3 . The incident energy of the neutrons was 3.4 MeV, the momentum transfer Q being 0.2 - 2.5 A -1 . A significant change in the order of the liquid has been registrated. Compressibility and electrical conductivity were derived from the structure factors and compared with the direct measured quantities, showing a good agreement. Further interpretation of the data was done by means of a hard core and a square well potential. Using these models it was already possible to get some information about the interactions between the rubidium atoms. A more exact calculation with a modified STLS model and a pseudopotential leads to a good description of the measured S(Q). In order to describe at high temperatures S(Q) for smaller values a new term had to be added to the pseudopotential. (orig.) [de

Influence of increasing nuclear charge on the Rydberg spectra of Xe, Cs+, and Ba++: Correlation, term dependence, and autoionization

International Nuclear Information System (INIS)

Hill, W.T. III; Cheng, K.T.; Johnson, W.R.; Lucatorto, T.B.; McIlrath, T.J.; Sugar, J.

1982-01-01

The first experimental-theoretical study of Rydberg autoionizing resonances along an isoelectronic sequence is presented. This analysis demonstrates the intimate connection between electron-electron correlation, term-dependence, and autoionization and underscores the power of multichannel quantum defect theory in analyzing complex spectra

Ionization of H Rydberg atoms

International Nuclear Information System (INIS)

Hillermier, C.F.; Bluemental, R.; Smilansky, U.

1991-07-01

Concepts from the theory of transient chaos are applied to study the classical ionization process of one dimensional model of kicked hydrogen Rydberg atoms. The phase-space dynamics is represented by a mapping T which is proved to be hyperbolic. The fraction of atoms not ionized after time t, P B (t), decays asymptotically according to P B (t)∼t -α with α ∼ 1.65. The observed algebraic decay, which seems to contradict the hyperbolicity of T, is explained by (i) the symbolic dynamics of T consists of a countably infinite number of symbols and (ii) the invariant manifold of phase-space points which never ionize is an anomalously scaling fractal. Therefore, the one-dimensional kicked hydrogen atom provides a counterexample to the hypothesis that algebraic decay marks regular dynamics, whereas hyperbolic systems decay exponentially. The algebraic decay is reproduced by an analytically solvable diffusion model which predicts α = 3/2. Replacing zero-width δ-kicks by smooth finite-width pulses, the mapping T is no longer completely hyperbolic, and a subset of phase-space is regular. For this case we observe that P B (t) shows a transition between two power-law decays with α ∼ 1.65 for short times and α ∼ 2.1 for long times where the effect of the regular domain is felt. (author)

Competition between font face="Symbol">Lfont>- and V-type transitions in interference stabilization of Rydberg atoms.

Science.gov (United States)

Fedorov, M; Poluektov, N

1998-01-19

The problem of Interference Stabilization of Rydberg atoms is considered. Two kinds of Raman-type transitions can be responsible for the effect: L-type transitions via the continuum and V-type transitions via lower resonant atomic levels. The main distinctions between L- and V- stabilization are described. The conditions under which each of these two effects can exist are found and discussed.

Dipole-dipole interactions in a hot atomic vapor and in an ultracold gas of Rydberg atoms

Science.gov (United States)

Sautenkov, V. A.; Saakyan, S. A.; Bronin, S. Ya; Klyarfeld, A. B.; Zelener, B. B.; Zelener, B. V.

2018-01-01

In our paper ideal and non-ideal gas media of neutral atoms are analyzed. The first we discuss a dipole broadening of atomic transitions in excited dilute and dense metal vapors. Then the theoretical studies of the dipole-dipole interactions in dense ultracold gas of Rydberg atoms are considered. Possible future experiments on a base of our experimental arrangement are suggested.

Lifetime measurements of highly excited Rydberg states of strontium. Pt. 1

International Nuclear Information System (INIS)

Kunze, S.; Hohmann, R.; Kluge, H.J.; Lantzsch, J.; Monz, L.; Stenner, J.; Stratmann, K.; Wendt, K.; Zimmer, K.

1993-01-01

Lifetimes of Rydberg states of triplet-series 5s ns 3 S 1 with n=19-23, 35 and 5s nd 3 D 3 with n=18-20, 23-28 in the spectrum of neutral strontium have been determined. Observation of the exponential decay after excitation by a pulsed laser in a fast atomic beam and subsequent state-selective field ionization was employed. The lifetimes of the states of the 3 S 1 -series show the expected n* 3 dependence on the effective principal quantum number, while the 3 D 3 -series is disturbed by configuration mixing. Furthermore, state re-populations induced by black-body radiation have been observed. (orig.)

Microwave spectroscopy of the 1 s n p P3J fine structure of high Rydberg states in 4He

Science.gov (United States)

Deller, A.; Hogan, S. D.

2018-01-01

The 1 s n p P3J fine structure of high Rydberg states in helium has been measured by microwave spectroscopy of single-photon transitions from 1 s n s S31 levels in pulsed supersonic beams. For states with principal quantum numbers in the range from n =34 to 36, the J =0 →2 and J =1 →2 fine structure intervals were both observed. For values of n between 45 and 51 only the larger J =0 →2 interval was resolved. The experimental results are in good agreement with theoretical predictions. Detailed characterization of residual uncanceled electric and magnetic fields in the experimental apparatus and calculations of the Stark and Zeeman structures of the Rydberg states in weak fields were used to quantify systematic contributions to the uncertainties in the measurements.

Analysis of high-n dielectronic Rydberg satellites in the spectra of Na-like Zn XX and Mg-like Zn XIX

International Nuclear Information System (INIS)

Fournier, K.B.; Faenov, A.Ya.; Pikuz, T.A.; Magunov, A.I.; Skobelev, I.Yu.; Flora, F.; Bollanti, S.; Di Lazzaro, P.; Murra, D.; Belyaev, V.S.; Vinogradov, V.I.; Kyrilov, A.S.; Matafonov, A.P.; Francucci, M.; Martellucci, S.; Petrocelli, G.

2004-01-01

We have observed spectra from highly charged zinc ions in a variety of laser-produced plasmas. Spectral features that are Na- and Mg-like satellites to high-n Rydberg transitions in the Ne-like Zn XXI spectrum are analyzed and modeled. Identifications and analysis are made by comparison with highly accurate atomic structure calculations and steady state collisional-radiative models. Each observed Zn XX and Zn XIX feature comprises up to ≅2 dozen individual transitions, these transitions are excited principally by dielectronic recombination through autoionizing levels in Na- and Mg-like Zn 19+ and Zn 18+ . We find these satellites to be ubiquitous in laser-produced plasmas formed by lasers with pulse lengths that span four orders of magnitude, from 1 ps to ≅10 ns. The diagnostic potential of these Rydberg satellite lines is demonstrated

Splitting of an electromagnetically induced transparency window of a cascade system with 133Cs Rydberg atoms in a static magnetic field

International Nuclear Information System (INIS)

Bao Shanxia; Yang Wenguang; Zhang Hao; Zhang Linjie; Zhao Jianming; Jia Suotang

2015-01-01

We investigate the electromagnetically induced transparency (EIT) of 133 Cs vapor at the room temperature in a magnetic field. In a cascade three-level system involved Rydberg state, two collinearly counter-propagating and orthogonally linear-polarized laser fields act on cascaded two transitions, 6S 1/2 → 6P 3/2 and 6P 3/2 ↔ 47D 5/2 , respectively. The EIT window become broadening and split into several sub-EIT windows when the magnetic field is applied. The dependences of splitting shape and intervals of sub-EIT windows on magnetic field are measured experimentally and compared with the theoretical calculation considering the different magnetic effects on ground state, low excited state and Rydberg state. The splitting intervals of sub-EIT windows are well consistent with theoretical calculation. (author)

The rate coefficients for the processes of (n - n')-mixing in collisions of Rydberg atoms H*(n) with H(1s) atoms

International Nuclear Information System (INIS)

Mihajlov, A A; Ignjatovic, Lj M; Djuric, Z; Ljepojevic, N N

2004-01-01

This paper presents the results of semi-classical calculations of rate coefficients of (n - n')-mixing processes in collisions of Rydberg atoms H*(n) with H(1s) atoms. These processes have been modelled by the mechanism of the resonant energy exchange within the electron component of the H*(n) + H collisional system. The calculations of the rate coefficients, based on this model, were performed for the series of principal quantum numbers, n and n', and atomic, T a , and electronic, T e , temperatures. It was shown that these processes can be of significant influence on the populations of Rydberg atoms in weakly ionized plasmas (ionization degree ∼ -4 ), and therefore have to be included in appropriate models of such plasmas

Dynamics of solvation and desolvation of rubidium attached to He nanodroplets

Energy Technology Data Exchange (ETDEWEB)

Vangerow, J. von; John, O.; Stienkemeier, F.; Mudrich, M., E-mail: mudrich@physik.uni-freiburg.de [Physikalisches Institut, Universität Freiburg, 79104 Freiburg (Germany)

2015-07-21

The real-time dynamics of photoexcited and photoionized rubidium (Rb) atoms attached to helium (He) nanodroplets is studied by femtosecond pump-probe mass spectrometry. While excited Rb atoms in the perturbed 6p-state (Rb{sup *}) desorb off the He droplets, Rb{sup +} photoions tend to sink into the droplet interior when created near the droplet surface. The transition from Rb{sup +} solvation to full Rb{sup *} desorption is found to occur at a delay time τ ∼ 600 fs for Rb{sup *} in the 6pΣ-state and τ ∼ 1200 fs for the 6pΠ-state. Rb{sup +}He ions are found to be created by directly exciting bound Rb{sup *}He exciplex states as well as by populating bound Rb{sup +}He-states in a photoassociative ionization process.

Time-resolved Fourier-transform infrared emission spectroscopy of Au in the 1800-4000-cm(-1) region: Rydberg transitions

Czech Academy of Sciences Publication Activity Database

Civiš, Svatopluk; Matulková, Irena; Cihelka, Jaroslav

2010-01-01

Roč. 81, č. 1 (2010), 012510 ISSN 1050-2947 R&D Projects: GA AV ČR IAA400400705; GA AV ČR KAN100500652 Institutional research plan: CEZ:AV0Z40400503 Keywords : spectroscopy * Rydberg transitions * theoretical chemistry Subject RIV: CF - Physical ; Theoretical Chemistry Impact factor: 2.861, year: 2010

Microwave multiphoton excitation of helium Rydberg atoms: The analogy with atomic collisions

International Nuclear Information System (INIS)

van de Water, W.; van Leeuwen, K.A.H.; Yoakum, S.; Galvez, E.J.; Moorman, L.; Bergeman, T.; Sauer, B.E.; Koch, P.M.

1989-01-01

We study multiphoton transitions in helium Rydberg atoms subjected to a microwave electric field of fixed frequency but varying intensity. For each principal quantum number in the range n=25--32, the n 3 S to n 3 (L>2), n=25--32, transition probability exhibits very sharp structures as a function of the field amplitude. Their positions could be reproduced precisely using a Floquet Hamiltonian for the interaction between atom and field. Their shapes are determined by the transients of field turn-on and turn-off in a way that makes a close analogy with the theory of slow atomic collisions

Rydberg states in a microwave field: regularity and chaos; Atomes de rydberg en champ micro-onde: regularite et chaos

Energy Technology Data Exchange (ETDEWEB)

Buchleitner, A

1993-12-15

We develop a theoretical formalism which provides a powerful tool for the detailed numerical analysis of the interaction of three-dimensional hydrogen atoms with an intense radiation field. The application of this approach to the microwave ionization of Rydberg states of hydrogen provides the most realistic numerical experiments ever made in this area. A thorough analysis of ionization signals and thresholds, of level dynamics and of the phase space projections of associated wave functions is provided for a one-dimensional model of the atom. The comparison to the ionization of three-dimensional atoms confirms the validity of the one-dimensional model for extended initial states and, hence, dynamical localization theory, as far as the ionization threshold is concerned. Three classes of three-dimensional initial states with distinct symmetries are identified and they appear to be more or less adapted to the symmetries of the eigenstates of the microwave problem. 'Scarred' wavefunctions of the three-dimensional hydrogen atom exposed to microwave field are shown. Finally, the dynamics of a circular state in a microwave and in an intense laser field are compared. (author)

Population coherent control of Rydberg potassium atom via adiabatic passage

International Nuclear Information System (INIS)

Jiang Li-Juan; Zhang Xian-Zhou; Jia Guang-Rui; Zhang Yong-Hui; Xia Li-Hua

2013-01-01

The time-dependent multilevel approach (TDMA) and B-spline expansion technique are used to study the coherent population transfer between the quantum states of a potassium atom by a single frequency-chirped microwave pulse. The Rydberg potassium atom energy levels of n = 6–15, l = 0–5 states in zero field are calculated and the results are in good agreement with other theoretical values. The time evolutions of the population transfer of the six states from n = 70 to n = 75 in different microwave fields are obtained. The results show that the coherent control of the population transfer from the lower states to the higher ones can be accomplished by optimizing the microwave pulse parameters. (atomic and molecular physics)

Detailed Balance of Thermalization Dynamics in Rydberg-Atom Quantum Simulators.

Science.gov (United States)

Kim, Hyosub; Park, YeJe; Kim, Kyungtae; Sim, H-S; Ahn, Jaewook

2018-05-04

Dynamics of large complex systems, such as relaxation towards equilibrium in classical statistical mechanics, often obeys a master equation that captures essential information from the complexities. Here, we find that thermalization of an isolated many-body quantum state can be described by a master equation. We observe sudden quench dynamics of quantum Ising-like models implemented in our quantum simulator, defect-free single-atom tweezers in conjunction with Rydberg-atom interaction. Saturation of their local observables, a thermalization signature, obeys a master equation experimentally constructed by monitoring the occupation probabilities of prequench states and imposing the principle of the detailed balance. Our experiment agrees with theories and demonstrates the detailed balance in a thermalization dynamics that does not require coupling to baths or postulated randomness.

Detailed Balance of Thermalization Dynamics in Rydberg-Atom Quantum Simulators

Science.gov (United States)

Kim, Hyosub; Park, YeJe; Kim, Kyungtae; Sim, H.-S.; Ahn, Jaewook

2018-05-01

Dynamics of large complex systems, such as relaxation towards equilibrium in classical statistical mechanics, often obeys a master equation that captures essential information from the complexities. Here, we find that thermalization of an isolated many-body quantum state can be described by a master equation. We observe sudden quench dynamics of quantum Ising-like models implemented in our quantum simulator, defect-free single-atom tweezers in conjunction with Rydberg-atom interaction. Saturation of their local observables, a thermalization signature, obeys a master equation experimentally constructed by monitoring the occupation probabilities of prequench states and imposing the principle of the detailed balance. Our experiment agrees with theories and demonstrates the detailed balance in a thermalization dynamics that does not require coupling to baths or postulated randomness.

Theory of collisional excitation transition between Rydberg states of atoms. Non-inertial mechanism

International Nuclear Information System (INIS)

Kaulakys, B.P.

1982-01-01

The transitions between highly states of an atom due to the collision of its core with another atom are considered. The cross sections of the change of highly excited electron angular momentum, in the case of the transitions when the main quantum number is constant, are expressed in terms of transport cross sections of the perturbing atom scattering on the ion of Rydberg atom. It is shown that the cross sections of the momentum mixing at thermal rapidities are lower than the cross sections of the atom-ion elastic scattering

Chemical reaction dynamics of Rydberg atoms with neutral molecules: A comparison of molecular-beam and classical trajectory results for the H(n)+D2→HD+D(n') reaction

International Nuclear Information System (INIS)

Song Hui; Dai Dongxu; Wu Guorong; Wang, C.-C.; Harich, Steven A.; Hayes, Michael Y.; Wang Xiuyan; Gerlich, Dieter; Yang Xueming; Skodje, Rex T.

2005-01-01

Recent molecular-beam experiments have probed the dynamics of the Rydberg-atom reaction, H(n)+D 2 →HD+D(n) at low collision energies. It was discovered that the rotationally resolved product distribution was remarkably similar to a much more limited data set obtained at a single scattering angle for the ion-molecule reaction H + +D 2 →D + +HD. The equivalence of these two problems would be consistent with the Fermi-independent-collider model (electron acting as a spectator) and would provide an important new avenue for the study of ion-molecule reactions. In this work, we employ a classical trajectory calculation on the ion-molecule reaction to facilitate a more extensive comparison between the two systems. The trajectory simulations tend to confirm the equivalence of the ion+molecule dynamics to that for the Rydberg-atom+molecule system. The theory reproduces the close relationship of the two experimental observations made previously. However, some differences between the Rydberg-atom experiments and the trajectory simulations are seen when comparisons are made to a broader data set. In particular, the angular distribution of the differential cross section exhibits more asymmetry in the experiment than in the theory. The potential breakdown of the classical model is discussed. The role of the 'spectator' Rydberg electron is addressed and several crucial issues for future theoretical work are brought out

Chemical aspects of rubidium uranium sulphate for its use as a chemical standard for uranium

International Nuclear Information System (INIS)

Singh Mudher, K.D.; Khandekar, R.R.; Krishnan, K.; Jayadevan, N.C.; Sood, D.D.

1989-01-01

Rb 2 U(SO 4 ) 3 , a double sulphate of rubidium and uranium(IV) has been prepared and investigated for its use as a chemical standard for uranium. The compound can be easily prepared and crystallised in a pure form. The results of physico-chemical characterisation on preparation of 5-10 g. lots are described in this report. These studies suggest that the compound is anhydrous, stoichiometric, stable to atmospheric effects and easily soluble in acids and thus satisfies most of the criteria for a primary standard. (author). 13 refs., 4 figs., 6 tabs

Crystal structure of the low-temperature forms of cesium and rubidium orthophosphates

International Nuclear Information System (INIS)

Voronin, V.I.; Proskurina, N.V.; Goshchitskij, B.N.; Berger, I.F.; Sheptyakov, D.V.; Burmakin, E.I.; Stroev, S.S.; Shekhtman, G.Sh.

2008-01-01

Making use of the neutron diffraction data base Rietveld method one for the first time determined and made more clear the crystal structure of the low-temperature modifications of Cs 3 PO 4 cesium and Rb 3 PO 4 rubidium orthophosphates. Cs 3 PO 4 and Rb 3 PO 4 were found to be isostructural one as to K 3 PO 4 . The structure is a rhombic one (Pnma, Z=4 sp.gr.) with the following elementary cell parameters: a = 1.23177(6) nm, b=0.88948(4) nm, c=0.64197(3) nm and a = 1.17362(2) nm, b=0.81046(1) nm, c=0.615167(9) nm for Cs 3 PO 4 and Rb 3 PO 4 respectively [ru

The rate coefficients for the processes of (n - n')-mixing in collisions of Rydberg atoms H*(n) with H(1s) atoms

Energy Technology Data Exchange (ETDEWEB)

Mihajlov, A A [Institute of Physics, PO Box 57, 11001 Belgrade (Serbia and Montenegro); Ignjatovic, Lj M [Institute of Physics, PO Box 57, 11001 Belgrade (Serbia and Montenegro); Djuric, Z [Silvaco Data Systems, Compass Point, St Ives PE27 5JL (United Kingdom); Ljepojevic, N N [Silvaco Data Systems, Compass Point, St Ives PE27 5JL (United Kingdom)

2004-11-28

This paper presents the results of semi-classical calculations of rate coefficients of (n - n')-mixing processes in collisions of Rydberg atoms H*(n) with H(1s) atoms. These processes have been modelled by the mechanism of the resonant energy exchange within the electron component of the H*(n) + H collisional system. The calculations of the rate coefficients, based on this model, were performed for the series of principal quantum numbers, n and n', and atomic, T{sub a}, and electronic, T{sub e}, temperatures. It was shown that these processes can be of significant influence on the populations of Rydberg atoms in weakly ionized plasmas (ionization degree {approx}<10{sup -4}), and therefore have to be included in appropriate models of such plasmas.

Influence of modulation frequency in rubidium cell frequency standards

Science.gov (United States)

Audoin, C.; Viennet, J.; Cyr, N.; Vanier, J.

1983-01-01

The error signal which is used to control the frequency of the quartz crystal oscillator of a passive rubidium cell frequency standard is considered. The value of the slope of this signal, for an interrogation frequency close to the atomic transition frequency is calculated and measured for various phase (or frequency) modulation waveforms, and for several values of the modulation frequency. A theoretical analysis is made using a model which applies to a system in which the optical pumping rate, the relaxation rates and the RF field are homogeneous. Results are given for sine-wave phase modulation, square-wave frequency modulation and square-wave phase modulation. The influence of the modulation frequency on the slope of the error signal is specified. It is shown that the modulation frequency can be chosen as large as twice the non-saturated full-width at half-maximum without a drastic loss of the sensitivity to an offset of the interrogation frequency from center line, provided that the power saturation factor and the amplitude of modulation are properly adjusted.

Theoretical analyses of an injection-locked diode-pumped rubidium vapor laser.

Science.gov (United States)

Cai, He; Gao, Chunqing; Liu, Xiaoxu; Wang, Shunyan; Yu, Hang; Rong, Kepeng; An, Guofei; Han, Juhong; Zhang, Wei; Wang, Hongyuan; Wang, You

2018-04-02

Diode-pumped alkali lasers (DPALs) have drawn much attention since they were proposed in 2001. The narrow-linewidth DPAL can be potentially applied in the fields of coherent communication, laser radar, and atomic spectroscopy. In this study, we propose a novel protocol to narrow the width of one kind of DPAL, diode-pumped rubidium vapor laser (DPRVL), by use of an injection locking technique. A kinetic model is first set up for an injection-locked DPRVL with the end-pumped configuration. The laser tunable duration is also analyzed for a continuous wave (CW) injection-locked DPRVL system. Then, the influences of the pump power, power of a master laser, and reflectance of an output coupler on the output performance are theoretically analyzed. The study should be useful for design of a narrow-linewidth DPAL with the relatively high output.

Rubidium mobility in the apple-tree and autoradiography as an aid in measuring the distribution and spread of the root-system

International Nuclear Information System (INIS)

Katana, H.; Kuehn, W.

1974-01-01

Investigations were made on the usability of rubidium-86 for measuring the distribution and spread of the root system of fruit trees. The tracer techniques developed so far in horticulture are not applicable for various reasons. Therefore, a new method of autoradiography was developed. The results of the preliminary investigations are very promising

Stark effect in Rydberg states of helium and barium

International Nuclear Information System (INIS)

Lahaije, C.T.W.

1989-01-01

This thesis, which deals with the effect of an electric field up to moderate field strengths on atoms with two valence electrons outside closed shells, in casu helium and barium, contains chapter in which the linear Stark effect in the 1 snp 1, 3 p Rydberg states of helium (n around 40) has been studied in a CW laser-atomic beam experiment. The evolution of the angular momentum manifolds into the n-mixing regime was followed and avoided level crossings were observed. Stark manifolds were also calculated by diagonalization of the complete energy matrix in the presence of an electric field. It turned out to be necessary to include up to five n-values in the calculations already at moderate values of the field to reproduce the data within the experimental accuracy (a few MHz), especially in the regime of the avoided crossings. (author). 147 refs.; 30 figs.; 8 tabs

Energy-level repulsion by spin-orbit coupling in two-dimensional Rydberg excitons

Science.gov (United States)

Stephanovich, V. A.; Sherman, E. Ya.; Zinner, N. T.; Marchukov, O. V.

2018-05-01

We study the effects of Rashba spin-orbit coupling on two-dimensional Rydberg exciton systems. Using analytical and numerical arguments we demonstrate that this coupling considerably modifies the wave functions and leads to a level repulsion that results in a deviation from the Poissonian statistics of the adjacent level distance distribution. This signifies the crossover to nonintegrability of the system and hints at the possibility of quantum chaos emerging. Such behavior strongly differs from the classical realization, where spin-orbit coupling produces highly entangled, chaotic electron trajectories in an exciton. We also calculate the oscillator strengths and show that randomization appears in the transitions between states with different total momenta.

The composition of the saturated vapor and enthalpies of dimerization of rubidium and cesium pivalates

International Nuclear Information System (INIS)

Khoretonenko, N.M.; Rykov, A.N.; Korenev, Yu.M.

1998-01-01

The rubidium and cesium pivalates sublimation processes are studied through the Knudsen effusion method with the mass-spectral analysis of the gaseous phase composition. It is established that MPiv and M 2 Piv 2 and in small amounts M 3 Piv 3 and M 4 Piv 4 constitute the basic components in the saturated vapour of the rubidium and cesium pivalates. Sublimation enthalpies (kJ/mole) of monomers Δ S H T 0 =163.5±7.2 and dimers Δ S H T 0 (Cs 2 Piv 2 )-192.1±9.6 are determined. Dissociation enthalpies (kJ/mole) of the M 2 Piv 2 dimers by the second(2) and the third (3) laws of thermodynamics: Δ D H T 0 (Cs 2 Piv 2 )=137.1±5.4(2), Δ D H T 0 (Rb 2 Piv 2 )=138.2±10.2 (3); Δ D H T 0 (Cs 2 Piv 2 )-134.9±9.3 (2), Δ D H T 0 (Cs 2 Piv 2 )=136.8±10.8 (3) are calculated. Temperature dependence equations (210-300 deg C of partial pressures (Pa) of the MPiv, M 2 Piv 2 molecules: InP(RbPiv)=-(20099±674)/T+34.6±1.2; InP(Rb 2 Piv 2 )=-(23707±734)/T+40.4±1.4; InP(CsPiv)=-(19666±866)/T+34.1±1.6; InP(Cs 2 Piv 2 )=-(23106±1155)/T+39.5±2.1 are obtained

A heated vapor cell unit for dichroic atomic vapor laser lock in atomic rubidium.

Science.gov (United States)

McCarron, Daniel J; Hughes, Ifan G; Tierney, Patrick; Cornish, Simon L

2007-09-01

The design and performance of a compact heated vapor cell unit for realizing a dichroic atomic vapor laser lock (DAVLL) for the D(2) transitions in atomic rubidium is described. A 5 cm long vapor cell is placed in a double-solenoid arrangement to produce the required magnetic field; the heat from the solenoid is used to increase the vapor pressure and correspondingly the DAVLL signal. We have characterized experimentally the dependence of important features of the DAVLL signal on magnetic field and cell temperature. For the weaker transitions both the amplitude and gradient of the signal are increased by an order of magnitude.

A heated vapor cell unit for dichroic atomic vapor laser lock in atomic rubidium

International Nuclear Information System (INIS)

McCarron, Daniel J.; Hughes, Ifan G.; Tierney, Patrick; Cornish, Simon L.

2007-01-01

The design and performance of a compact heated vapor cell unit for realizing a dichroic atomic vapor laser lock (DAVLL) for the D 2 transitions in atomic rubidium is described. A 5 cm long vapor cell is placed in a double-solenoid arrangement to produce the required magnetic field; the heat from the solenoid is used to increase the vapor pressure and correspondingly the DAVLL signal. We have characterized experimentally the dependence of important features of the DAVLL signal on magnetic field and cell temperature. For the weaker transitions both the amplitude and gradient of the signal are increased by an order of magnitude

Generation of narrow-band polarization-entangled photon pairs at a rubidium D1 line

International Nuclear Information System (INIS)

Tian Long; Li Shujing; Yuan Haoxiang; Wang Hai

2016-01-01

Using the process of cavity-enhanced spontaneous parametric down-conversion (SPDC), we generate a narrow-band polarization-entangled photon pair resonant on the rubidium (Rb) D1 line (795 nm). The degenerate single-mode photon pair is selected by multiple temperature controlled etalons. The linewidth of generated polarization-entangled photon pairs is 15 MHz which matches the typical atomic memory bandwidth. The measured Bell parameter for the polarization-entangled photons S = 2.73 ± 0.04 which violates the Bell-CHSH inequality by ∼18 standard deviations. The presented entangled photon pair source could be utilized in quantum communication and quantum computing based on quantum memories in atomic ensemble. (author)

Two-electron excitation to Rydberg levels in fast I6+ on hydrogen collisions

International Nuclear Information System (INIS)

Liao, C.; Hagmann, S.; Zouros, T.J.M.; Montenegro, E.C.; Toth, G.; Richard, P.; Grabbe, S.; Bhalla, C.P.

1995-01-01

The emission of electrons in the forward direction in collisions of 0.3 MeV/u I 6+ with H 2 has been studied, and strong autoionization peaks are observed on the shoulder of the cusp peak. The energies of these autoionization lines in the projectile rest frame are determined by high-resolution electron spectroscopy. Using the electron projectile final charge state coincidence technique, we probe different collision mechanisms, which create continuum electrons that are slow in the projectile rest frame. We conclude that the observed autoionization lines are due to two electron excitation to projectile Rydberg levels. (orig.)

Rydberg states in a microwave field: regularity and chaos; Atomes de rydberg en champ micro-onde: regularite et chaos

Energy Technology Data Exchange (ETDEWEB)

Buchleitner, A

1993-12-15

We develop a theoretical formalism which provides a powerful tool for the detailed numerical analysis of the interaction of three-dimensional hydrogen atoms with an intense radiation field. The application of this approach to the microwave ionization of Rydberg states of hydrogen provides the most realistic numerical experiments ever made in this area. A thorough analysis of ionization signals and thresholds, of level dynamics and of the phase space projections of associated wave functions is provided for a one-dimensional model of the atom. The comparison to the ionization of three-dimensional atoms confirms the validity of the one-dimensional model for extended initial states and, hence, dynamical localization theory, as far as the ionization threshold is concerned. Three classes of three-dimensional initial states with distinct symmetries are identified and they appear to be more or less adapted to the symmetries of the eigenstates of the microwave problem. 'Scarred' wavefunctions of the three-dimensional hydrogen atom exposed to microwave field are shown. Finally, the dynamics of a circular state in a microwave and in an intense laser field are compared. (author)

AEgIS at ELENA: outlook for physics with a pulsed cold antihydrogen beam

Science.gov (United States)

Doser, M.; Aghion, S.; Amsler, C.; Bonomi, G.; Brusa, R. S.; Caccia, M.; Caravita, R.; Castelli, F.; Cerchiari, G.; Comparat, D.; Consolati, G.; Demetrio, A.; Di Noto, L.; Evans, C.; Fanì, M.; Ferragut, R.; Fesel, J.; Fontana, A.; Gerber, S.; Giammarchi, M.; Gligorova, A.; Guatieri, F.; Haider, S.; Hinterberger, A.; Holmestad, H.; Kellerbauer, A.; Khalidova, O.; Krasnický, D.; Lagomarsino, V.; Lansonneur, P.; Lebrun, P.; Malbrunot, C.; Mariazzi, S.; Marton, J.; Matveev, V.; Mazzotta, Z.; Müller, S. R.; Nebbia, G.; Nedelec, P.; Oberthaler, M.; Pacifico, N.; Pagano, D.; Penasa, L.; Petracek, V.; Prelz, F.; Prevedelli, M.; Rienaecker, B.; Robert, J.; Røhne, O. M.; Rotondi, A.; Sandaker, H.; Santoro, R.; Smestad, L.; Sorrentino, F.; Testera, G.; Tietje, I. C.; Widmann, E.; Yzombard, P.; Zimmer, C.; Zmeskal, J.; Zurlo, N.

2018-03-01

The efficient production of cold antihydrogen atoms in particle traps at CERN's Antiproton Decelerator has opened up the possibility of performing direct measurements of the Earth's gravitational acceleration on purely antimatter bodies. The goal of the AEgIS collaboration is to measure the value of g for antimatter using a pulsed source of cold antihydrogen and a Moiré deflectometer/Talbot-Lau interferometer. The same antihydrogen beam is also very well suited to measuring precisely the ground-state hyperfine splitting of the anti-atom. The antihydrogen formation mechanism chosen by AEgIS is resonant charge exchange between cold antiprotons and Rydberg positronium. A series of technical developments regarding positrons and positronium (Ps formation in a dedicated room-temperature target, spectroscopy of the n=1-3 and n=3-15 transitions in Ps, Ps formation in a target at 10 K inside the 1 T magnetic field of the experiment) as well as antiprotons (high-efficiency trapping of ?, radial compression to sub-millimetre radii of mixed ? plasmas in 1 T field, high-efficiency transfer of ? to the antihydrogen production trap using an in-flight launch and recapture procedure) were successfully implemented. Two further critical steps that are germane mainly to charge exchange formation of antihydrogen-cooling of antiprotons and formation of a beam of antihydrogen-are being addressed in parallel. The coming of ELENA will allow, in the very near future, the number of trappable antiprotons to be increased by more than a factor of 50. For the antihydrogen production scheme chosen by AEgIS, this will be reflected in a corresponding increase of produced antihydrogen atoms, leading to a significant reduction of measurement times and providing a path towards high-precision measurements. This article is part of the Theo Murphy meeting issue `Antiproton physics in the ELENA era'.

Searching for an oscillating massive scalar field as a dark matter candidate using atomic hyperfine frequency comparisons

OpenAIRE

Hees, A.; Guéna, J.; Abgrall, M.; Bize, S.; Wolf, P.

2016-01-01

We use six years of accurate hyperfine frequency comparison data of the dual rubidium and caesium cold atom fountain FO2 at LNE-SYRTE to search for a massive scalar dark matter candidate. Such a scalar field can induce harmonic variations of the fine structure constant, of the mass of fermions and of the quantum chromodynamic mass scale, which will directly impact the rubidium/caesium hyperfine transition frequency ratio. We find no signal consistent with a scalar dark matter candidate but pr...

Lifetime measurements of highly excited Rydberg states of strontium. Pt. 1

Energy Technology Data Exchange (ETDEWEB)

Kunze, S.; Hohmann, R.; Kluge, H.J.; Lantzsch, J.; Monz, L.; Stenner, J.; Stratmann, K.; Wendt, K.; Zimmer, K. (Mainz Univ. (Germany). Inst. fuer Physik)

1993-06-01

Lifetimes of Rydberg states of triplet-series 5s ns[sup 3]S[sub 1] with n=19-23, 35 and 5s nd[sup 3]D[sub 3] with n=18-20, 23-28 in the spectrum of neutral strontium have been determined. Observation of the exponential decay after excitation by a pulsed laser in a fast atomic beam and subsequent state-selective field ionization was employed. The lifetimes of the states of the [sup 3]S[sub 1]-series show the expected n*[sup 3] dependence on the effective principal quantum number, while the [sup 3]D[sub 3]-series is disturbed by configuration mixing. Furthermore, state re-populations induced by black-body radiation have been observed. (orig.).

Semiclassical analysis of quantum localization of the periodically kicked Rydberg atom

International Nuclear Information System (INIS)

Yoshida, S.; Persson, E.; Burgdoerfer, J.; Grossmann, F.

2004-01-01

The periodically kicked Rydberg atom displays quantum localization, features of which depend on the orientation and strength of the unidirectional kicks. They include scarring of the wave function, localization by cantori, and exponential localization in the regime of strong perturbation resembling dynamical localization. Using the semiclassical Herman-Kluk propagator we investigate the degree to which semiclassical dynamics can mimic quantum localization. While the semiclassical approximation has difficulties to reproduce the scarred wave functions, the exponential tail which is a typical signature of the dynamical localization is well represented in the case of strong classical diffusion. Also the localization by broken tori is observed in the semiclassical recurrence probability for short times but the deviation from the corresponding quantum dynamics becomes more pronounced for the long-time evolution

Study of the phase transition in lithium potassium rubidium sulfate system

Science.gov (United States)

Hamed, A. E.; Abd. El-Aziz, Y. M.; Madi, N. K.; Kassem, M. E.

1998-10-01

Specific heat, Cp, measurements have been performed in lithium potassium rubidium sulfate, (Li 0.5- x/2 K 0.5- x/2 Rb x) 2SO 4, system in a wide range of Rb 2SO 4 content ( x) ( x=0 up to x=10%). Measurements were made between 300 and 800 K with special attention paid to the phase transition at 708 K. It is shown that for small contents, ( x), ( x=0.2 up to x=2%) quantitative changes in the temperature dependence of specific heat Cp( T) around the transition point, T1, are observed. A larger content, x, results in essential changes in the critical behavior of Cp( T) and a considerable change in the phase transition accompanied by a progressive decrease in the thermodynamic parameters. The ratios of the Landau expansion coefficients change as the content of Rb 2SO 4 increases.

Engineering Photon-Photon Interactions within Rubidium-Filled Waveguides

Science.gov (United States)

Perrella, C.; Light, P. S.; Vahid, S. Afshar; Benabid, F.; Luiten, A. N.

2018-04-01

Strong photon-photon interactions are a required ingredient for deterministic two-photon optical quantum logic gates. Multiphoton transitions in dense atomic vapors have been shown to be a promising avenue for producing such interactions. The strength of a multiphoton interaction can be enhanced by conducting the interaction in highly confined geometries such as small-cross-section optical waveguides. We demonstrate, both experimentally and theoretically, that the strength of such interactions scale only with the optical mode diameter, d , not d2 as might be initially expected. This weakening of the interaction arises from atomic motion inside the waveguides. We create an interaction between two optical signals, at 780 and 776 nm, using the 5 S1 /2→5 D5 /2 two-photon transition in rubidium vapor within a range of hollow-core fibers with different core sizes. The interaction strength is characterized by observing the absorption and phase shift induced on the 780-nm beam, which is in close agreement with theoretical modeling that accounts for the atomic motion inside the fibers. These observations demonstrate that transit-time effects upon multiphoton transitions are of key importance when engineering photon-photon interactions within small-cross-section waveguides that might otherwise be thought to lead to enhanced optical nonlinearity through increased intensities.

Dynamical localization in the 3-D kicked Rydberg atom

International Nuclear Information System (INIS)

Persson, E.; Yoshida, S.; Tong, X.-M.; Reinhold, C.; Burgdoerfer, J.

2001-01-01

Full text: The dynamical localization for the 3D periodically kicked Rydberg atom is analyzed. For the 1D kicked atom, earlier work shows dynamical localization as the quantum suppression of classically fast ionization associated with unbounded chaotic trajectories. The corresponding wave functions localize around unstable periodic orbits. For the experimental observation, the crucial question is the dependence of the dynamical localization on the dimension. As the first step, we simulate the full 3D evolution of an extreme parabolic initial state elongated in the direction of the unidirectional kicks. We compare this simulation with the 1D model and find signatures of localization also in 3D. We further examine the dependence of quantum localization on the parabolic quantum number of the initial state. In the limit of high kick frequencies, the origin of the localization can be understood in terms of Stark states in the average field. We discuss conditions for where an experimental observation of the localization is most likely. (author)

Sound speed of isobaric heat capacity in the saturated and superheated vapour of cesium, rubidium and potassium

International Nuclear Information System (INIS)

Novikov, I.I.; Roschupkin, V.V.

1985-01-01

The paper reviews the work carried out on the thermodynamic properties of alkali metal vapours. The most systematic investigations concern the sound velocity measurements for saturated and superheated vapours of caesium, for saturated vapour of rubidium, and for superheated vapour of potassium. The Joule-Thompson coefficient has been studied in caesium vapour, and the isobaric heat capacity of potassium vapour has also been examined. The experimental methods for all these experiments are described, and the data obtained are presented in tabular form. (U.K.)

Rydberg gas theory of a glow discharge plasma: I. Application to the electrical behaviour of a fast flowing glow discharge plasma.

Science.gov (United States)

Mason, Rod S; Mitchell, David J; Dickinson, Paul M

2010-04-21

Current-voltage (I-V) curves have been measured, independent of the main discharge, for electricity passing through the steady state fast flowing 'afterglow' plasma of a low power dc glow discharge in Ar. Voltage profiles along the axial line of conduction have been mapped using fixed probes and potentiometry, and the mass spectra of cations emerging from the downstream sampling Cone, also acting as a probe anode, were recorded simultaneously. Floating double probe experiments were also carried out. The electrical behavior is consistent with the well established I-V characteristics of such discharges, but does not comply with classical plasma theory predictions. The plasma decays along the line of conduction, with a lifetime of approximately 1 ms, despite carrying a steady state current, and its potential is below that of the large surface area anode voltage; a situation which cannot exist in the presence of a conventional free ion-electron plasma, unless the electron temperature is super cold. Currents, large by comparison with the main discharge current, and independent of it, are induced to flow through the downstream plasma, from the Anode (acting as a cathode) to the anodic ion exit Cone, induced by electron impact ionisation at the anode, but without necessarily increasing the plasma density. It appears to be conducted by direct charge transfer between a part of the anode surface (acting as cathode to the auxiliary circuit) and the plasma, without secondary electron emission or heating, which suggests the direct involvement of Rydberg atom intermediates. The reaction energy defect (= the work function of the electrode surface) fits with the plasma potential threshold observed for the cathodic reaction to occur. A true free ion-electron plasma is readily detected by the observation of cations at the anode surface, when induced at the downstream anode, at high bias voltages, by the electron impact ionisation in the boundary region. In contrast to the classical

Wavelength mismatch effect in electromagnetically induced absorption

International Nuclear Information System (INIS)

Bharti, Vineet; Wasan, Ajay; Natarajan, Vasant

2016-01-01

We present a theoretical investigation of the phenomenon of electromagnetically induced absorption (EIA) in a 4-level system consisting of vee and ladder subsystems. The four levels are coupled using one weak probe field, and two strong control fields. We consider an experimental realization using energy levels of Rb. This necessitates dealing with different conditions of wavelength mismatch—near-perfect match where all three wavelengths are approximately equal; partial mismatch where the wavelength of one control field is less than the other fields; and complete mismatch where all three wavelengths are unequal. We present probe absorption profiles with Doppler averaging at room temperature to account for experiments in a room temperature Rb vapor cell. Our analysis shows that EIA resonances can be studied using Rydberg states excited with diode lasers. - Highlights: • Wavelength mismatch effect is investigated in electromagnetically induced absorption (EIA). • An experimental realization of 4-level vee + ladder system using energy levels of rubidium atom is presented. • EIA resonances are studied under different conditions of wavelength mismatch. • Possibility of observation of EIA using Rydberg states excited with diode lasers.

Wavelength mismatch effect in electromagnetically induced absorption

Energy Technology Data Exchange (ETDEWEB)

Bharti, Vineet [Department of Physics, Indian Institute of Science, Bangalore 560012 (India); Wasan, Ajay [Department of Physics, Indian Institute of Technology, Roorkee 247667 (India); Natarajan, Vasant [Department of Physics, Indian Institute of Science, Bangalore 560012 (India)

2016-07-15

We present a theoretical investigation of the phenomenon of electromagnetically induced absorption (EIA) in a 4-level system consisting of vee and ladder subsystems. The four levels are coupled using one weak probe field, and two strong control fields. We consider an experimental realization using energy levels of Rb. This necessitates dealing with different conditions of wavelength mismatch—near-perfect match where all three wavelengths are approximately equal; partial mismatch where the wavelength of one control field is less than the other fields; and complete mismatch where all three wavelengths are unequal. We present probe absorption profiles with Doppler averaging at room temperature to account for experiments in a room temperature Rb vapor cell. Our analysis shows that EIA resonances can be studied using Rydberg states excited with diode lasers. - Highlights: • Wavelength mismatch effect is investigated in electromagnetically induced absorption (EIA). • An experimental realization of 4-level vee + ladder system using energy levels of rubidium atom is presented. • EIA resonances are studied under different conditions of wavelength mismatch. • Possibility of observation of EIA using Rydberg states excited with diode lasers.

Dielectronic recombination rate coefficients of initially rubidium-like tungsten

International Nuclear Information System (INIS)

Wu, Z.; Zhang, Y.; Fu, Y.; Dong, C.; Surzhykov, A.; Fritzsche, S.

2015-01-01

Dielectric recombination (DR) is a dominant electron recombination process in plasmas. Tungsten ions are expected to be prominent impurities in fusion plasmas so the knowledge of DR rate coefficient of tungsten ions is important to model fusion plasmas. Ab initio calculations of DR rate coefficients of initially rubidium-like W 37+ ions have been performed for the electron temperatures from 1 eV to 5*10 4 eV, by using the Flexible Atomic Code based on the relativistic configuration-interaction method. Special attention has been paid to the partial contributions to total DR rate coefficients as associated with the excitation of individual subshells. A detailed comparison of the calculations shows that the excitation from 4p subshell dominates total DR rate coefficients followed by the excitations from 4s and 4d subshells, while the contribution of excitations from 3l (l = s, p, d) subshells becomes important only at high temperatures. Besides, it is found that the electron excitations associated with Δn = 0, 1 dominate at low-temperature plasmas, however, the excitations associated with Δn ≥ 2 become non-negligible at high-temperature ones

Structural, Mechanical and Thermodynamic Properties under Pressure Effect of Rubidium Telluride: First Principle Calculations

Directory of Open Access Journals (Sweden)

Bidai K.

2017-06-01

Full Text Available First-principles density functional theory calculations have been performed to investigate the structural, elastic and thermodynamic properties of rubidium telluride in cubic anti-fluorite (anti-CaF2-type structure. The calculated ground-state properties of Rb2Te compound such as equilibrium lattice parameter and bulk moduli are investigated by generalized gradient approximation (GGA-PBE that are based on the optimization of total energy. The elastic constants, Young’s and shear modulus, Poisson ratio, have also been calculated. Our results are in reasonable agreement with the available theoretical and experimental data. The pressure dependence of elastic constant and thermodynamic quantities under high pressure are also calculated and discussed.

Semiclassical study of the collision of a highly excited Rydberg atom with the molecules HF and HCl

International Nuclear Information System (INIS)

Kimura, M.; Lane, N.F.

1990-01-01

The semiclassical impact-parameter method is applied to the processes of state changing and energy transfer in the collision of a highly excited Rydberg atom (n≥20) with the polar molecules HF and HCl. The relative motion of the molecule and atomic nucleus is taken to be rectilinear; the electron-molecule and ion core-molecule interactions are represented by cutoff dipole forms. Cross sections for transitions involving quantum numbers n and l of the atom and rotational quantum number j of the molecule are obtained for a range of collision energies and initial atomic and molecular states. Comparisons are made with the results of earlier classical studies and with the quantum-mechanical impulse approximation. Collision rates are calculated and compared with experimental values for l mixing and n and j changing. The agreement between experiment and theory is shown to be satisfactory, within the uncertainties of both the measurements and the theory. Cases of agreement and disagreement between various theories are examined. One finding of the present work is that the quantum-mechanical impulse approximation appears to significantly overestimate the values of various state-changing cross sections when the internal energy defect is small. The validity of the impulse approximation for collisions of Rydberg atoms with polar molecules is discussed

Theoretical investigation of output features of a diode-pumped rubidium vapor laser

Science.gov (United States)

Wang, You; Cai, He; Zhang, Wei; Xue, Liangping; Wang, Hongyuan; Han, Juhong

2014-02-01

In the recent years, diode-pumped alkali lasers (DPALs) have been paid many attentions because of their excellent performances. In fact, the characteristics of a DPAL strongly depend on the physical features of buffer gases. In this report, we selected a diode-pumped rubidium vapor laser (DPRVL), which is an important type among three common DPALs, to investigate how the characteristics of a DPRVL are affected by different conditions. The results signify that the population ratio of two excitation energy-levels are close to that corresponding to thermal equilibrium as the pressure of buffer gases and the temperature of a vapor cell become higher. It has been found that quenching of the upper levels cannot be simply ignored especially for the case of weak pump. The conclusions are thought to be helpful for the configuration design of an end-pumped DPAL.

The role of Rydberg and continuum levels in computing high harmonic generation spectra of the hydrogen atom using time-dependent configuration interaction

International Nuclear Information System (INIS)

Luppi, Eleonora; Head-Gordon, Martin

2013-01-01

We study the role of Rydberg bound-states and continuum levels in the field-induced electronic dynamics associated with the High-Harmonic Generation (HHG) spectroscopy of the hydrogen atom. Time-dependent configuration-interaction (TD-CI) is used with very large atomic orbital (AO) expansions (up to L= 4 with sextuple augmentation and off-center functions) to describe the bound Rydberg levels, and some continuum levels. To address the lack of ionization losses in TD-CI with finite AO basis sets, we employed a heuristic lifetime for energy levels above the ionization potential. The heuristic lifetime model is compared against the conventional atomic orbital treatment (infinite lifetimes), and a third approximation which is TD-CI using only the bound levels (continuum lifetimes go to zero). The results suggest that spectra calculated using conventional TD-CI do not converge with increasing AO basis set size, while the zero lifetime and heuristic lifetime models converge to qualitatively similar spectra, with implications for how best to apply bound state electronic structure methods to simulate HHG. The origin of HHG spectral features including the cutoff and extent of interference between peaks is uncovered by separating field-induced coupling between different types of levels (ground state, bound Rydberg levels, and continuum) in the simulated electronic dynamics. Thus the origin of deviations between the predictions of the semi-classical three step model and the full simulation can be associated with particular physical contributions, which helps to explain both the successes and the limitations of the three step model

The impact of prompt gamma compensation on myocardial blood flow measurements with rubidium-82 dynamic PET.

Science.gov (United States)

Armstrong, Ian S; Memmott, Matthew J; Tonge, Christine M; Arumugam, Parthiban

2018-04-01

Rubidium-82 myocardial perfusion imaging is a well-established technique for assessing myocardial ischemia. With continuing interest on myocardial blood flow (MBF) and myocardial flow reserve (MFR) measurements, there is a requirement to fully appreciate the impact of technical aspects of the process. One such factor for rubidium-82 is prompt gamma compensation (PGC). This study aims to assess the impact of PGC on MBF and MFR calculated from dynamic Rb-82 data. Dynamic rest and stress images were acquired on a Siemens Biograph mCT and reconstructed with and without PGC in 50 patients (29 male). MBF and MFR were measured in the three main coronary territories as well as globally. With PGC, statistically significant reductions in MBF were observed in LAD (-6.9%), LCx (-4.8%), and globally (-6.5%) but only in obese patients. Significant increases in MBF were observed in RCA (+6.4%) in only nonobese patients. In very obese patients, differences of up to 40% in MBF were observed between PGC and non-PGC images. In nearly all cases, similar PGC differences were observed at stress and rest so there were no significant differences in MFR; however, in a small number of very obese patients, differences in excess of 20% were observed. PGC results in statistically significant changes in MBF, with the greatest reductions observed in the LAD and LCx territories of obese patients. In most cases, the impact on stress and rest data is of similar relative magnitudes and changes to MFR are small.

Phase diagram of Rydberg atoms with repulsive van der Waals interaction

International Nuclear Information System (INIS)

Osychenko, O. N.; Astrakharchik, G. E.; Boronat, J.; Lutsyshyn, Y.; Lozovik, Yu. E.

2011-01-01

We report a quantum Monte Carlo calculation of the phase diagram of bosons interacting with a repulsive inverse sixth power pair potential, a model for assemblies of Rydberg atoms in the local van der Waals blockade regime. The model can be parametrized in terms of just two parameters, the reduced density and temperature. Solidification happens to the fcc phase. At zero temperature, the transition density is found with the diffusion Monte Carlo method at density ρ=3.9 ((ℎ/2π) 2 /mC 6 ) 3/4 , where C 6 is the strength of the interaction. The solidification curve at nonzero temperature is studied with the path-integral Monte Carlo approach and is compared with transitions in corresponding harmonic and classical crystals. Relaxation mechanisms are considered in relation to present experiments.

Ionization photophysics and Rydberg spectroscopy of diacetylene

KAUST Repository

Schwell, Martin

2012-11-01

Photoionization of diacetylene was studied using synchrotron radiation over the range 8-24 eV, with photoelectron-photoion coincidence (PEPICO) and threshold photoelectron-photoion coincidence (TPEPICO) techniques. Mass spectra, ion yields, total and partial ionization cross-sections were measured. The adiabatic ionization energy of diacetylene was determined as IE ad=(10.17±0.01) eV, and the appearance energy of the principal fragment ion C4H+ as AE=(16.15±0.03) eV. Calculated appearance energies of other fragment ions were used to infer aspects of dissociation pathways forming the weaker fragment ions C+ 4, C3H+, C+3 and C 4H+. Structured autoionization features observed in the PEPICO spectrum of diacetylene in the 11-13 eV region were assigned to vibrational components of three new Rydberg series, R1(nsσg, n=4-11), R2(ndσg, n=4-7) and R3(ndδg, n=4-6) converging to the A2Πu state of the cation, and to a new series R01(nsσg, n=3) converging to the B\\' 2Σ+u state of the cation. The autoionization mechanisms and their consistence with specific selection rules are discussed. © 2012 Taylor and Francis.

Ionization photophysics and Rydberg spectroscopy of diacetylene

KAUST Repository

Schwell, Martin; Bé nilan, Yves; Fray, Nicolas; Gazeau, Marie Claire; Es-sebbar, Et-touhami; Gaie-Levrel, Franç ois; Champion, Norbert; Leach, Sydney Sydney

2012-01-01

Photoionization of diacetylene was studied using synchrotron radiation over the range 8-24 eV, with photoelectron-photoion coincidence (PEPICO) and threshold photoelectron-photoion coincidence (TPEPICO) techniques. Mass spectra, ion yields, total and partial ionization cross-sections were measured. The adiabatic ionization energy of diacetylene was determined as IE ad=(10.17±0.01) eV, and the appearance energy of the principal fragment ion C4H+ as AE=(16.15±0.03) eV. Calculated appearance energies of other fragment ions were used to infer aspects of dissociation pathways forming the weaker fragment ions C+ 4, C3H+, C+3 and C 4H+. Structured autoionization features observed in the PEPICO spectrum of diacetylene in the 11-13 eV region were assigned to vibrational components of three new Rydberg series, R1(nsσg, n=4-11), R2(ndσg, n=4-7) and R3(ndδg, n=4-6) converging to the A2Πu state of the cation, and to a new series R01(nsσg, n=3) converging to the B' 2Σ+u state of the cation. The autoionization mechanisms and their consistence with specific selection rules are discussed. © 2012 Taylor and Francis.

Positronium in the AEgIS experiment: study on its emission from nanochanneled samples and design of a new apparatus for Rydberg excitations

CERN Document Server

Di Noto, Lea

This experimental thesis has been done in the framework of AEgIS (Antimatter Experiment: Gravity, Interferometry, Spectroscopy), an experiment installed at CERN, whose primary goal is the measurement of the Earth's gravitational acceleration on anti-hydrogen. The antiatoms will be produced by the charge exchange reaction, where a cloud of Ps in Rydberg states interacts with cooled trapped antiprotons. Since the charge exchange cross section depends on Ps velocity and quantum number, the velocity distribution of Ps emitted by a positron-positronium converter as well as its excitation in Rydberg states have to be studied and optimized. In this thesis Ps cooling and emission into vacuum from nanochannelled silicon targets was studied by performing Time of Flight measurements with a dedicated apparatus conceived to receive the slow positron beam as produced at the Trento laboratory or at the NEPOMUC facility at Munich. Measurements were done by varying the positron implantation energy, the sample temperature and ...

Semi-classical description of Rydberg atoms in strong, single-cycle electromagnetic pulses

International Nuclear Information System (INIS)

Jensen, R.V.; Sanders, M.M.

1993-01-01

Recent experimental measurements of the excitation and ionization of Rydberg atoms by single-cycle, electromagnetic pulses have revealed a variety of novel features. Because many quantum states are strongly coupled by the broadband radiation in the short pulse, the traditional methods of quantum mechanics are inadequate to account for the experimental results. We have therefore developed a semi-classical description of the interaction of both hydrogenic and non-hydrogenic atoms with single-cycle pulses of intense, electromagnetic radiation which is based on the strong correspondence theory of Percival and Richards. This theory, which was originally introduced for the description of strong atomic collisions, accounts for some of the surprising features of the experimental measurements and provides new predictions for future experimental studies

Identification of X-ray spectra in the Na-like to O-like rubidium ions in the range of 3.8-7.3 Angstroms

International Nuclear Information System (INIS)

Denis-Petit, D.; Bonnet, T.; Hannachi, F.; Gobet, F.; Tarisien, M.; Versteegen, M.; Comet, M.; Gosselin, G.; Meot, V.; Morel, P.; Pain, J.Ch.; Gilleron, F.; Frank, A.; Bagnoud, V.; Blazevic, A.; Dorchies, F.; Peyrusse, O.; Cayzac, W.; Roth, M.

2014-01-01

The X-rays emitted by a rubidium plasma source created by the PHELIX laser at an intensity of about 6*10"1"4 W/cm"2 were studied. The lines have been measured using Bragg crystals in the wavelength range between 3.8 and 7.3 Angstroms and identified by means of a numerical method developed to describe highly charged rubidium ions in LTE plasma. The experimental plasma temperature, density and charge state distributions have been estimated using non-LTE codes such as CHIVAS and AVERROES. The LTE plasma temperature and density used in the calculations are those allowing to reproduce the calculated NLTE charge state distribution. In order to optimize the use of computational resources, a criterion is established to select the configurations contributing most to the spectra among all those obtained in detailed level accounting based on the MCDF code. Seventy Rb-X-rays have been identified among which forty-nine are reported for the first time. The capabilities of our method are demonstrated by the good agreement of our identifications with previously published data when available. (authors)

Detection of cold pain, cold allodynia and cold hyperalgesia in freely behaving rats

Directory of Open Access Journals (Sweden)

Woolf Clifford J

2005-12-01

Full Text Available Abstract Background Pain is elicited by cold, and a major feature of many neuropathic pain states is that normally innocuous cool stimuli begin to produce pain (cold allodynia. To expand our understanding of cold induced pain states we have studied cold pain behaviors over a range of temperatures in several animal models of chronic pain. Results We demonstrate that a Peltier-cooled cold plate with ± 1°C sensitivity enables quantitative measurement of a detection withdrawal response to cold stimuli in unrestrained rats. In naïve rats the threshold for eliciting cold pain behavior is 5°C. The withdrawal threshold for cold allodynia is 15°C in both the spared nerve injury and spinal nerve ligation models of neuropathic pain. Cold hyperalgesia is present in the spared nerve injury model animals, manifesting as a reduced latency of withdrawal response threshold at temperatures that elicit cold pain in naïve rats. We also show that following the peripheral inflammation produced by intraplantar injection of complete Freund's adjuvant, a hypersensitivity to cold occurs. Conclusion The peltier-cooled provides an effective means of assaying cold sensitivity in unrestrained rats. Behavioral testing of cold allodynia, hyperalgesia and pain will greatly facilitate the study of the neurobiological mechanisms involved in cold/cool sensations and enable measurement of the efficacy of pharmacological treatments to reduce these symptoms.

Asymptotically exact expression for the energies of the 3Se Rydberg series in a two-electron system

International Nuclear Information System (INIS)

Ivanov, I.A.; Bromley, M.W.J.; Mitroy, J.

2002-01-01

The 1sns 3 S e Rydberg series in a two-electron system with the charge of the nucleus, Z≅1, is treated by means of the quantum-defect theory. Comparison with configuration interaction calculations suggests that the quantum-defect expression for the energy levels becomes asymptotically exact as Z→1. This provides an analytic description of the disappearance of the 1sns 3 S e bound states when Z approaches the critical value of 1

A Controlled-Phase Gate via Adiabatic Rydberg Dressing of Neutral Atoms

Science.gov (United States)

Keating, Tyler; Deutsch, Ivan; Cook, Robert; Biederman, Grant; Jau, Yuan-Yu

2014-05-01

The dipole blockade effect between Rydberg atoms is a promising tool for quantum information processing in neutral atoms. So far, most efforts to perform a quantum logic gate with this effect have used resonant laser pulses to excite the atoms, which makes the system particularly susceptible to decoherence through thermal motional effects. We explore an alternative scheme in which the atomic ground states are adiabatically ``dressed'' by turning on an off-resonant laser. We analyze the implementation of a CPHASE gate using this mechanism and find that fidelities of >99% should be possible with current technology, owing primarily to the suppression of motional errors. We also discuss how such a scheme could be generalized to perform more complicated, multi-qubit gates; in particular, a simple generalization would allow us to perform a Toffoli gate in a single step.

l- and n-changing collisions during interaction of a pulsed beam of Li Rydberg atoms with CO2

Science.gov (United States)

Dubreuil, B.; Harnafi, M.

1989-07-01

The pulsed Li atomic beam produced in our experiment is based on controlled transversely-excited-atmospheric CO2 laser-induced ablation of a Li metal target. The atomic beam is propagated in vacuum or in CO2 gas at low pressure. Atoms in the beam are probed by laser-induced fluorescence spectroscopy. This allows the determination of time-of-flight and velocity distributions. Li Rydberg states (n=5-13) are populated in the beam by two-step pulsed-laser excitation. The excited atoms interact with CO2 molecules. l- and n-changing cross sections are deduced from the time evolution of the resonant or collision-induced fluorescence following this selective excitation. l-changing cross sections of the order of 104 AṦ are measured; they increase with n as opposed to the plateau observed for Li* colliding with a diatomic molecule. This behavior is qualitatively well explained in the framework of the free-electron model. n-->n' changing processes with large cross sections (10-100 AṦ) are also observed even in the case of large electronic energy change (ΔEnn'>103 cm-1). These results can be interpreted in terms of resonant-electronic to vibrational energy transfers between Li Rydberg states and CO2 vibrational modes.

Rydberg states in a microwave field: regularity and chaos

International Nuclear Information System (INIS)

Buchleitner, A.

1993-12-01

We develop a theoretical formalism which provides a powerful tool for the detailed numerical analysis of the interaction of three-dimensional hydrogen atoms with an intense radiation field. The application of this approach to the microwave ionization of Rydberg states of hydrogen provides the most realistic numerical experiments ever made in this area. A thorough analysis of ionization signals and thresholds, of level dynamics and of the phase space projections of associated wave functions is provided for a one-dimensional model of the atom. The comparison to the ionization of three-dimensional atoms confirms the validity of the one-dimensional model for extended initial states and, hence, dynamical localization theory, as far as the ionization threshold is concerned. Three classes of three-dimensional initial states with distinct symmetries are identified and they appear to be more or less adapted to the symmetries of the eigenstates of the microwave problem. 'Scarred' wavefunctions of the three-dimensional hydrogen atom exposed to microwave field are shown. Finally, the dynamics of a circular state in a microwave and in an intense laser field are compared. (author)

Lithium, rubidium and cesium ion removal using potassium iron(III) hexacyanoferrate(II) supported on polymethylmethacrylate

International Nuclear Information System (INIS)

Shabana Taj; Din Muhammad; Ashraf Chaudhry, M.; Muhammad Mazhar

2011-01-01

Potassium iron(III) hexacyanoferrate(II) supported on poly methyl methacrylate, has been developed and investigated for the removal of lithium, rubidium and cesium ions. The material is capable of sorbing maximum quantities of these ions from 5.0, 2.5 and 4.5 M HNO 3 solutions respectively. Sorption studies, conducted individually for each metal ion, under optimized conditions, demonstrated that it was predominantly physisorption in the case of lithium ion while shifting to chemisorption with increasing ionic size. Distribution coefficient (K d ) values followed the order Cs + > Rb + > Li + at low concentrations of metal ions. Following these findings Cs + can preferably be removed from 1.5 to 5 M HNO 3 nuclear waste solutions. (author)

Analysis of the X-ray emission spectra of copper, germanium and rubidium plasmas produced at the Phelix laser facility

Science.gov (United States)

Comet, M.; Pain, J.-C.; Gilleron, F.; Piron, R.; Denis-Petit, D.; Méot, V.; Gosselin, G.; Morel, P.; Hannachi, F.; Gobet, F.; Tarisien, M.; Versteegen, M.

2017-03-01

We present the analysis of X-ray emission spectra of copper, germanium and rubidium plasmas measured at the Phelix laser facility. The laser intensity was around 6×1014 W.cm-2. The analysis is based on the hypothesis of an homogeneous plasma in local thermodynamic equilibrium using an effective temperature. This temperature is deduced from hydrodynamic simulations and collisional-radiative computations. Spectra are then calculated using the LTE opacity codes OPAMCDF and SCO-RCG and compared to experimental data.

Experimental study of linear magnetic dichroism in photoionization satellite transitions of atomic rubidium

International Nuclear Information System (INIS)

Jaenkaelae, K.; Alagia, M.; Feyer, V.; Richter, R.; Prince, K. C.

2011-01-01

Laser orientation in the initial state has been used to study the properties of satellite transitions in inner-shell photoionization of rubidium atoms. The linear magnetic dichroism in the angular distribution (LMDAD) has been utilized to probe the continuum waves of orbital angular momentum conserving monopole, and angular momentum changing conjugate satellites, accompanying the 4p ionization of atomic Rb. We show experimentally that LMDAD of both types of satellite transitions is nonzero and that LMDAD of monopole satellites, measured as a function of photon energy, mimics the LMDAD of direct photoionization, whereas the LMDAD of conjugate transitions deviates drastically from that trend. The results indicate that conjugate transitions cannot be described theoretically without explicit inclusion of electron-electron interaction. The present data can thus be used as a very precise test of current models for photoionization.

Fabrication and characterization of rubidium/formamidinium-incorporated methylammonium-lead-halide perovskite solar cells

Science.gov (United States)

Kato, Masataka; Suzuki, Atsushi; Ohishi, Yuya; Tanaka, Hiroki; Oku, Takeo

2018-01-01

Fabrication and characterization of perovskite solar cells using mesoporous TiO2 as an electron transporting layer and 2,2',7,7'-tetrakis-(N,N-di-4-methoxyphenylamino)-9,9'-spirobifluorene as a hole-transporting layer were performed for improving the photovoltaic performance. Additive effects of formamidinium (FA), rubidium (Rb), chlorine (Cl) and bromine (Br) into the methylammonium-lead-halide perovskite crystal on the photovoltaic properties and microstructures were investigated. The photovoltaic parameters of short-circuit current density, conversion efficiency, the surface morphology and domain in the perovskite crystal were characterized. The slight addition of FACl and RbBr to the CH3NH3PbI3 crystal provided homogeneous microstructures with the dispersed crystal domains, which improved the photovoltaic performance. The excess addition of Cl to the perovskite crystal caused nanorod-like crystals, which degraded the photovoltaic performance.

The production and investigation of cold antihydrogen atoms

International Nuclear Information System (INIS)

Pittner, H.

2005-04-01

This work reports on experiments in which antihydrogen atoms have been produced in cryogenic Penning traps from antiproton and positron plasmas by two different methods and on experiments that have been carried out subsequently in order to investigate the antihydrogen atoms. By the first method antihydrogen atoms have been formed during the process of positron cooling of antiprotons in so called nested Penning traps and detected via a field ionization method. A measurement of the state distribution has revealed that the antihydrogen atoms are formed in highly excited states. This suggests along with the high production rate that the antihydrogen atoms are formed by three-body recombination processes and subsequent collisional deexcitations. However current theory cannot yet account for the measured state distribution. Typical radii of the detected antihydrogen atoms lie in the range between 0.4 μm and 0.15 μm. The deepest bound antihydrogen atoms have radii below 0.1 μm.The kinetic energy of the weakest bound antihydrogen atoms has been measured to about 200 meV. By the second method antihydrogen atoms have been synthesized in charge-exchange processes. Lasers are used to produce a Rydberg cesium beam within the cryogenic Penning trap that collides with trapped positrons so that Rydberg positronium atoms are formed via charge-exchange reactions. The Rydberg positronium atoms that collide with nearby stored antiprotons form antihydrogen atoms in charge-exchange reactions. So far, 14±4 antihydrogen atoms have been detected background-free via a field-ionization method. The antihydrogen atoms produced via the two-step charge-exchange mechanism are expected to have a temperature of 4.2 K, the temperature of the antiprotons from which they are formed

Charge transfer rates for xenon Rydberg atoms at metal and semiconductor surfaces

Energy Technology Data Exchange (ETDEWEB)

Dunning, F.B. [Department of Physics and Astronomy, Rice University, MS 61, 6100 Main Street, Houston, TX 77005-1892 (United States)]. E-mail: fbd@rice.edu; Wethekam, S. [Institut fuer Physik der Humboldt-Universitaet zu Berlin, Newtonstr. 15, D-12489 Berlin (Germany); Dunham, H.R. [Department of Physics and Astronomy, Rice University, MS 61, 6100 Main Street, Houston, TX 77005-1892 (United States); Lancaster, J.C. [Department of Physics and Astronomy, Rice University, MS 61, 6100 Main Street, Houston, TX 77005-1892 (United States)

2007-05-15

Recent progress in the study of charge exchange between xenon Rydberg atoms and surfaces is reviewed. Experiments using Au(1 1 1) surfaces show that under appropriate conditions each incident atom can be detected as an ion. The ionization dynamics, however, are strongly influenced by the perturbations in the energies and structure of the atomic states that occur as the ion collection field is applied and as the atom approaches the surface. These lead to avoided crossings between different atomic levels causing the atom to successively assume the character of a number of different states and lose much of its initial identity. The effects of this mixing are discussed. Efficient surface ionization is also observed at Si(1 0 0) surfaces although the ion signal is influenced by stray fields present at the surface.

Nonlinear spectroscopy of the Rydberg atoms

International Nuclear Information System (INIS)

Delone, N.B.; Krajnov, V.P.; Shepelyanskij, D.L.

1984-01-01

The results of investigation into perturbation of Rydberg states (RS) of atoms in an outer alternating field (OAF) are discussed. Both highly excited states of hydrogen atom at the energy Esub(n)=-1/2n -2 (n>>1 - basic quantum number) and excited states of compound atoms with energy Esub(nl)=-1/2(n*) -2 where n*=n-delta sub(e)-effective basic quantum number, delta sub(e)-quantum defect, are implied by RS. Perturbation of atomic state in the OAF is determined not only by field strength E, but by its frequency ω as well. During OAF inclusion the initial state Esub(lambda) transits to quasienergetic at the energy Esub(lambda)(E)+-kω, where K=0, +-1, +-2, .... Solutions of the problem of quasienergetic level population is obtained only for some simple particular cases. A simple case, when a real multilevel atom is replaced by a model system comprising one bound electron state with the basic quantum number n-model of the insulated level (MIL) is considered. Conditions of MIL applicability are discussed. Estimation of critical OAF strength at which MIL approximation becomes faulty are discussed. It is stated that any consideration of RS perturbation in OAF claiming to exceeding MIL frames should comprise consideration of ionization processes. If one keeps to the frames of OAF; the strength of which is lower than the determined critical values then MIL is true and use of this model permits to correctly describe the main features of RS perturbation in an alternating field

Compact Optical Atomic Clock Based on a Two-Photon Transition in Rubidium

Science.gov (United States)

Martin, Kyle W.; Phelps, Gretchen; Lemke, Nathan D.; Bigelow, Matthew S.; Stuhl, Benjamin; Wojcik, Michael; Holt, Michael; Coddington, Ian; Bishop, Michael W.; Burke, John H.

2018-01-01

Extralaboratory atomic clocks are necessary for a wide array of applications (e.g., satellite-based navigation and communication). Building upon existing vapor-cell and laser technologies, we describe an optical atomic clock, designed around a simple and manufacturable architecture, that utilizes the 778-nm two-photon transition in rubidium and yields fractional-frequency instabilities of 4 ×10-13/√{τ (s ) } for τ from 1 to 10 000 s. We present a complete stability budget for this system and explore the required conditions under which a fractional-frequency instability of 1 ×10-15 can be maintained on long time scales. We provide a precise characterization of the leading sensitivities to external processes, including magnetic fields and fluctuations of the vapor-cell temperature and 778-nm laser power. The system is constructed primarily from commercially available components, an attractive feature from the standpoint of the commercialization and deployment of optical frequency standards.

Van-der-Waals interaction of atoms in dipolar Rydberg states

Science.gov (United States)

Kamenski, Aleksandr A.; Mokhnenko, Sergey N.; Ovsiannikov, Vitaly D.

2018-02-01

An asymptotic expression for the van-der-Waals constant C 6( n) ≈ -0.03 n 12 K p ( x) is derived for the long-range interaction between two highly excited hydrogen atoms A and B in their extreme Stark states of equal principal quantum numbers n A = n B = n ≫ 1 and parabolic quantum numbers n 1(2) = n - 1, n 2(1) = m = 0 in the case of collinear orientation of the Stark-state dipolar electric moments and the interatomic axis. The cubic polynomial K 3( x) in powers of reciprocal values of the principal quantum number x = 1/ n and quadratic polynomial K 2( y) in powers of reciprocal values of the principal quantum number squared y = 1/ n 2 were determined on the basis of the standard curve fitting polynomial procedure from the calculated data for C 6( n). The transformation of attractive van-der-Waals force ( C 6 > 0) for low-energy states n < 23 into repulsive force ( C 6 < 0) for all higher-energy states of n ≥ 23, is observed from the results of numerical calculations based on the second-order perturbation theory for the operator of the long-range interaction between neutral atoms. This transformation is taken into account in the asymptotic formulas (in both cases of p = 2, 3) by polynomials K p tending to unity at n → ∞ ( K p (0) = 1). The transformation from low- n attractive van-der-Waals force into high- n repulsive force demonstrates the gradual increase of the negative contribution to C 6( n) from the lower-energy two-atomic states, of the A(B)-atom principal quantum numbers n'A(B) = n-Δ n (where Δ n = 1, 2, … is significantly smaller than n for the terms providing major contribution to the second-order series), which together with the states of n″B(A) = n+Δ n make the joint contribution proportional to n 12. So, the hydrogen-like manifold structure of the energy spectrum is responsible for the transformation of the power-11 asymptotic dependence C 6( n) ∝ n 11of the low-angular-momenta Rydberg states in many-electron atoms into the power

AEgIS at ELENA: outlook for physics with a pulsed cold antihydrogen beam.

Science.gov (United States)

Doser, M; Aghion, S; Amsler, C; Bonomi, G; Brusa, R S; Caccia, M; Caravita, R; Castelli, F; Cerchiari, G; Comparat, D; Consolati, G; Demetrio, A; Di Noto, L; Evans, C; Fanì, M; Ferragut, R; Fesel, J; Fontana, A; Gerber, S; Giammarchi, M; Gligorova, A; Guatieri, F; Haider, S; Hinterberger, A; Holmestad, H; Kellerbauer, A; Khalidova, O; Krasnický, D; Lagomarsino, V; Lansonneur, P; Lebrun, P; Malbrunot, C; Mariazzi, S; Marton, J; Matveev, V; Mazzotta, Z; Müller, S R; Nebbia, G; Nedelec, P; Oberthaler, M; Pacifico, N; Pagano, D; Penasa, L; Petracek, V; Prelz, F; Prevedelli, M; Rienaecker, B; Robert, J; Røhne, O M; Rotondi, A; Sandaker, H; Santoro, R; Smestad, L; Sorrentino, F; Testera, G; Tietje, I C; Widmann, E; Yzombard, P; Zimmer, C; Zmeskal, J; Zurlo, N

2018-03-28

The efficient production of cold antihydrogen atoms in particle traps at CERN's Antiproton Decelerator has opened up the possibility of performing direct measurements of the Earth's gravitational acceleration on purely antimatter bodies. The goal of the AEgIS collaboration is to measure the value of g for antimatter using a pulsed source of cold antihydrogen and a Moiré deflectometer/Talbot-Lau interferometer. The same antihydrogen beam is also very well suited to measuring precisely the ground-state hyperfine splitting of the anti-atom. The antihydrogen formation mechanism chosen by AEgIS is resonant charge exchange between cold antiprotons and Rydberg positronium. A series of technical developments regarding positrons and positronium (Ps formation in a dedicated room-temperature target, spectroscopy of the n =1-3 and n =3-15 transitions in Ps, Ps formation in a target at 10 K inside the 1 T magnetic field of the experiment) as well as antiprotons (high-efficiency trapping of [Formula: see text], radial compression to sub-millimetre radii of mixed [Formula: see text] plasmas in 1 T field, high-efficiency transfer of [Formula: see text] to the antihydrogen production trap using an in-flight launch and recapture procedure) were successfully implemented. Two further critical steps that are germane mainly to charge exchange formation of antihydrogen-cooling of antiprotons and formation of a beam of antihydrogen-are being addressed in parallel. The coming of ELENA will allow, in the very near future, the number of trappable antiprotons to be increased by more than a factor of 50. For the antihydrogen production scheme chosen by AEgIS, this will be reflected in a corresponding increase of produced antihydrogen atoms, leading to a significant reduction of measurement times and providing a path towards high-precision measurements.This article is part of the Theo Murphy meeting issue 'Antiproton physics in the ELENA era'. © 2018 The Author(s).

A theoretical investigation of valence and Rydberg electronic states of acrolein

International Nuclear Information System (INIS)

Aquilante, Francesco; Barone, Vincenzo; Roos, Bjoern O.

2003-01-01

The main features of the ultraviolet spectrum of acrolein have been studied by a multireference perturbative treatment and by a time dependent density functional approach. The valence and Rydberg transition energies have been calculated and the assignment of the experimental bands has been clarified. The different relaxation trends of the three lowest singlet and triplet excited states have been analyzed by unconstrained geometry optimizations. This has allowed, in particular, the characterization of a twisted 3 (ππ*) state, which is crucial for the interesting photophysics and photochemistry of the acrolein molecule and, more generally, of the α,β-enones. Solvatochromic shifts in aqueous solution have been investigated using a combined discrete/continuum approach based on the so called polarizable continuum model. The experimental trends are well reproduced by this approach and a closer degeneracy in the triplet manifold has been detected in solution with respect to gas phase

Neutron powder diffraction and theory-aided structure refinement of rubidium and cesium ureate

Energy Technology Data Exchange (ETDEWEB)

Sterri, Kjersti B.; Deringer, Volker L.; Houben, Andreas; Jacobs, Philipp [RWTH Aachen Univ. (Germany). Inst. of Inorganic Chemistry; Kumar, Chogondahalli M.N. [Forschungszentrum Juelich GmbH, Juelich Centre for Neutron Science (JCNS), Outstation at SNS, Oak Ridge National Laboratory, Oak Ridge, TN (United States); Oak Ridge National Laboratory, TN (United States). Chemical and Engineering Materials Div.; Dronskowski, Richard [RWTH Aachen Univ. (Germany). Inst. of Inorganic Chemistry; RWTH Aachen Univ. (Germany). Juelich-Aachen Research Alliance (JARA-HPC)

2016-08-01

Urea (CN{sub 2}H{sub 4}O) is a fundamental biomolecule whose derivatives are abundant throughout chemistry. Among the latter, rubidium ureate (RbCN{sub 2}H{sub 3}O) and its cesium analog (CsCN{sub 2}H{sub 3}O) have been described only very recently and form the first structurally characterized salts of deprotonated urea. Here, we report on a neutron diffraction study on the aforementioned alkaline-metal ureates, which affords the positions for all hydrogen atoms (including full anisotropic displacement tensors) and thus allows us to gain fundamental insights into the hydrogen-bonding networks in the title compounds. The structure refinements of the experimental neutron data proceeded successfully using starting parameters from ab initio simulations of atomic positions and anisotropic displacement parameters. Such joint experimental-theoretical refinement procedures promise significant practical potential in cases where complex solids (organic, organometallic, framework materials) are studied by powder diffraction.

Exponential and nonexponential localization of the one-dimensional periodically kicked Rydberg atom

International Nuclear Information System (INIS)

Yoshida, S.; Reinhold, C. O.; Kristoefel, P.; Burgdoerfer, J.

2000-01-01

We investigate the quantum localization of the one-dimensional Rydberg atom subject to a unidirectional periodic train of impulses. For high frequencies of the train the classical system becomes chaotic and leads to fast ionization. By contrast, the quantum system is found to be remarkably stable. We identify for this system the coexistence of different localization mechanisms associated with resonant and nonresonant diffusion. We find for the suppression of nonresonant diffusion an exponential localization whose localization length can be related to the classical dynamics in terms of the ''scars'' of the unstable periodic orbits. We show that the localization length is determined by the energy excursion along the periodic orbits. The suppression of resonant diffusion along the sequence of photonic peaks is found to be nonexponential due to the presence of high harmonics in the driving force. (c) 2000 The American Physical Society

How cold is cold dark matter?

International Nuclear Information System (INIS)

Armendariz-Picon, Cristian; Neelakanta, Jayanth T.

2014-01-01

If cold dark matter consists of particles, these must be non-interacting and non-relativistic by definition. In most cold dark matter models however, dark matter particles inherit a non-vanishing velocity dispersion from interactions in the early universe, a velocity that redshifts with cosmic expansion but certainly remains non-zero. In this article, we place model-independent constraints on the dark matter temperature to mass ratio, whose square root determines the dark matter velocity dispersion. We only assume that dark matter particles decoupled kinetically while non-relativistic, when galactic scales had not entered the horizon yet, and that their momentum distribution has been Maxwellian since that time. Under these assumptions, using cosmic microwave background and matter power spectrum observations, we place upper limits on the temperature to mass ratio of cold dark matter today (away from collapsed structures). These limits imply that the present cold dark matter velocity dispersion has to be smaller than 54 m/s. Cold dark matter has to be quite cold, indeed

Cold Antimatter Plasmas, and Aspirations for Cold Antihydrogen

Science.gov (United States)

2002-06-24

UNCLASSIFIED Defense Technical Information Center Compilation Part Notice ADP012494 TITLE: Cold Antimatter Plasmas, and Aspirations for Cold...part numbers comprise the compilation report: ADP012489 thru ADP012577 UNCLASSIFIED Cold Antimatter Plasmas, and Aspirations for Cold Antihydrogen G...and positrons. The antiprotons come initially from the new Antiproton Decel- erator facility at CERN. Good control of such cold antimatter plasmas is

Effects of finite temperature on two-photon transitions in a Rydberg atom in a high-Q cavity

International Nuclear Information System (INIS)

Puri, R.R.; Joshi, A.

1989-01-01

The effects of cavity temperature on an effective two-level atom undergoing two-photon transitions in a high-Q cavity are investigated. The quantum statistical properties of the field and the dynamical properties of the atom in this case are studied and compared with those for an atom making one-photon transitions between the two levels. The analysis is based on the solution of the equation for the density matrix in the secular approximation which is known to be a valid approximation in the case of a Rydberg atom in a high-Q cavity. (orig.)

Generation of tunable coherent far-infrared radiation using atomic Rydberg states

International Nuclear Information System (INIS)

Bookless, W.

1980-12-01

A source of tunable far-infrared radiation has been constructed. The system has been operated at 91.6 cm -1 with a demonstrated tunability of .63 cm -1 . The system is based on a Rydberg state transition in optically pumped potassium vapor. The transition energy is tuned by the application of an electric field to the excited vapor. The transition wavelength and the shifted wavelength were detected and measured by the use of a Michelson interferometer and a liquid helium cooled Ga:Ge bolometer and the data was reduced using Fast Fourier transform techniques. Extensive spectroscopy was done on the potassium vapor to elucidate the depopulation paths and rates of the excited levels. Both theoretical and experimental results are presented to support the conclusions of the research effort. Additionally, possible alternative approaches to the population of the excited state are explored and recommendations are made for the future development of this source as well as the potential uses of it in molecular spectroscopy

Exciton Rydberg series in mono- and few-layer WS2

Science.gov (United States)

Chernikov, Alexey; Berkelbach, Timothy C.; Hill, Heather M.; Rigosi, Albert; Li, Yilei; Aslan, Özgur B.; Hybertsen, Mark S.; Reichman, David R.; Heinz, Tony F.

2014-03-01

Considered a long-awaited semiconducting analogue to graphene, the family of atomically thin transition metal dichalcogenides (TMDs) attracted intense interest in the scientific community due to their remarkable physical properties resulting from the reduced dimensionality. A fundamental manifestation of the two-dimensional nature is a strong increase in the Coulomb interaction. The resulting formation of tightly bound excitons plays a crucial role for a majority of optical and transport phenomena. In our work, we investigate the excitons in atomically thin TMDs by optical micro-spectroscopy and apply a microscopic, ab-initio theoretical approach. We observe a full sequence of excited exciton states, i.e., the Rydberg series, in the monolayer WS2, identifying tightly bound excitons with energies exceeding 0.3 eV - almost an order of magnitude higher than in the corresponding, three-dimensional crystal. We also find significant deviations of the excitonic properties from the conventional hydrogenic physics - a direct evidence of a non-uniform dielectric environment. Finally, an excellent quantitative agreement is obtained between the experimental findings and the developed theoretical approach.

Atomic spin resonance in a rubidium beam obliquely incident to a transmission magnetic grating

International Nuclear Information System (INIS)

Hatakeyama, A; Goto, K

2016-01-01

We studied atomic spin resonance induced by atomic motion in a spatially periodic magnetostatic field. A rubidium atomic beam, with a velocity of about 400 m s −1 , was obliquely incident to a transmission magnetic grating that produced a spatially periodic magnetic field. The magnetic grating was formed by a magnetic thin film on a polyimide substrate that had multiple slits at 150 μm intervals. The atoms experienced field oscillation, depending on their velocity and the field period when passing through the grating, and underwent magnetic resonance. Resonance spectra obtained with a perpendicular magnetization film were in clear contrast to ones obtained with an in-plane magnetization film. The former exhibited resonance peaks at odd multiples of the frequency, determined by the velocity over the period, while the latter had dips at the same frequencies. (paper)

Hypothermic general cold adaptation induced by local cold acclimation.

Science.gov (United States)

Savourey, G; Barnavol, B; Caravel, J P; Feuerstein, C; Bittel, J H

1996-01-01

To study relationships between local cold adaptation of the lower limbs and general cold adaptation, eight subjects were submitted both to a cold foot test (CFT, 5 degrees C water immersion, 5 min) and to a whole-body standard cold air test (SCAT, 1 degree C, 2 h, nude at rest) before and after a local cold acclimation (LCA) of the lower limbs effected by repeated cold water immersions. The LCA induced a local cold adaptation confirmed by higher skin temperatures of the lower limbs during CFT and a hypothermic insulative general cold adaptation (decreased rectal temperature and mean skin temperature P adaptation was related to the habituation process confirmed by decreased plasma concentrations of noradrenaline (NA) during LCA (P general cold adaptation was unrelated either to local cold adaptation or to the habituation process, because an increased NA during SCAT after LCA (P syndrome" occurring during LCA.

Thermodynamic Properties of Alkali Metal Hydroxides. Part II. Potassium, Rubidium, and Cesium Hydroxides

International Nuclear Information System (INIS)

Gurvich, L.V.; Bergman, G.A.; Gorokhov, L.N.; Iorish, V.S.; Leonidov, V.Y.; Yungman, V.S.

1997-01-01

The data on thermodynamic and molecular properties of the potassium, rubidium and cesium hydroxides have been collected, critically reviewed, analyzed, and evaluated. Tables of the thermodynamic properties [C p circ , Φ=-(G -H(0)/T, S, H -H(0), Δ f H, Δ f G)] of these hydroxides in the condensed and gaseous states have been calculated using the results of the analysis and some estimated values. The recommendations are compared with earlier evaluations given in the JANAF Thermochemical Tables and Thermodynamic Properties of Individual Substances. The properties considered are: the temperature and enthalpy of phase transitions and fusion, heat capacities, spectroscopic data, structures, bond energies, and enthalpies of formation at 298.15 K. The thermodynamic functions in solid, liquid, and gaseous states are calculated from T=0 to 2000 K for substances in condensed phase and up to 6000 K for gases. copyright 1997 American Institute of Physics and American Chemical Society

Magnetic resonance of rubidium atoms passing through a multi-layered transmission magnetic grating

International Nuclear Information System (INIS)

Nagata, Y; Kurokawa, S; Hatakeyama, A

2017-01-01

We measured the magnetic resonance of rubidium atoms passing through periodic magnetic fields generated by two types of multi-layered transmission magnetic grating. One of the gratings reported here was assembled by stacking four layers of magnetic films so that the direction of magnetization alternated at each level. The other grating was assembled so that the magnetization at each level was aligned. For both types of grating, the experimental results were in good agreement with our calculations. We studied the feasibility of extending the frequency band of the grating and narrowing its resonance linewidth by performing calculations. For magnetic resonance precision spectroscopy, we conclude that the multi-layered transmission magnetic grating can generate periodic fields with narrower linewidths at higher frequencies when a larger number of layers are assembled at a shorter period length. Moreover, the frequency band of this type of grating can potentially achieve frequencies of up to hundreds of PHz. (paper)

Structure determination, electronic and optical properties of rubidium holmium polyphosphate RbHo(PO3)4

Science.gov (United States)

Zhu, Jing; Chen, Hui; Wang, Yude; Guan, Hongtao; Xiao, Xuechun

2012-12-01

Structural, optical, and electronic properties of a new alkali metal-rare earth polyphosphate, RbHo(PO3)4, have been investigated by means of single-crystal X-ray diffraction, power X-ray diffraction, elemental analysis, and spectral measurement. RbHo(PO3)4 crystallizes in the monoclinic with space group P21/n and Z = 4. It is described as a three-dimensional (3D) architecture built up of PO4 double spiral chains and HoO8 polyhedra by corner-sharing. The 11-coordinated rubidium atoms are located in infinite tunnels. Additionally, in order to gain further insight into the relationship between property and structure of RbHo(PO3)4, theoretical calculation based on the density functional theory (DFT) was performed using the total-energy code CASTEP.

The world of quantum matter

CERN Multimedia

CERN. Geneva

2006-01-01

In my lecture series, I will present the recent spectacular advances in the field of quantum gases and macroscopic quantum physics. A variety of subjects will be covered including Bose condensates and degenerate Fermi gases, ultracold molecules and chemistry near absolute zero, Rydberg gases, single-atom manipulation, quantum information processing, as well as applications of cold atoms as precision targets. The topics of the lectures are: I. Physics near absolute zero II. Bose condensation and Fermi degeneracy III. Molecules, Rydberg gases and other exotic species IV. Single-atom manipulation, quantum information processing and ultracold atoms as targets in storage rings

Cold Stress

Science.gov (United States)

... Publications and Products Programs Contact NIOSH NIOSH COLD STRESS Recommend on Facebook Tweet Share Compartir Workers who ... cold environments may be at risk of cold stress. Extreme cold weather is a dangerous situation that ...

Nuclear structure studies of the neutron-rich Rubidium isotopes using Coulomb excitation

CERN Multimedia

Reiter, P; Blazhev, A A; Voulot, D; Meot, V H; Simpson, G S; Georgiev, G P; Gaudefroy, L; Roig, O

We propose to study the properties of odd-mass neutron-rich rubidium isotopes by the Coulomb-excitation technique, using the Miniball array coupled to the REX-ISOLDE facility. The results from similar measurements from the recent years (e.g. for the odd-mass and the odd-odd Cu isotopes, IS435) have shown the strong potential in such measurements for gaining information both for single-particle-like and collective states in exotic nuclei. Since there is practically no experimental information for excited states in the odd-mass Rb isotopes beyond $^{93}$Rb, the present study should be able to provide new data in a region of spherical ($^{93}$Rb and $^{95}$Rb) as well as well-deformed nuclei ($^{97}$Rb and $^{99}$Rb). Of particular interest is the rapid shape change that occurs when going from $^{95}$Rb (${\\varepsilon}_{2}$=0.06) to $^{97}$Rb (${\\varepsilon}_{2}$=0.3). These results should be of significant astrophysical interest as well, due to the close proximity of the r-process path.

Verification of the validity of the short-pulse approximation for one-dimensional Rydberg atoms

International Nuclear Information System (INIS)

Kopyciuk, T; Grajek, M

2011-01-01

In this paper, we investigate the short-pulse approximation (SPA) for one-dimensional Rydberg atoms. We analyse the limits that SPA has to fulfil in order to be applicable. These concern the shape, the duration and the displacement caused by the pulse. The correctness of SPA is tested by comparing the results obtained using SPA with a numerical solution of the set of time-dependent Schroedinger equations. We show that the limit for the displacement caused by the pulse is of greatest importance. Violation of the limit for the duration of the pulse is shown to lead to concurrent violation of the limit for the displacement. We also show that the shape of the pulse has no influence on the created wave packet.

Skeletal muscle blood flow in vivo: detection with rubidium-82 and effects of glucose, insulin, and exercise

International Nuclear Information System (INIS)

Mossberg, K.A.; Mullani, N.; Gould, K.L.; Taegtmeyer, H.

1987-01-01

In order to assess the effects of glucose, insulin, and exercise on skeletal muscle blood flow in vivo, we measured positron emission from the thigh muscle of anesthetized rabbits after simultaneous aortic bolus injection of 82 Rb and radiolabeled microspheres (15 micron diameter). Estimates of flow with 82 Rb were based on first-pass regional extraction of 82 Rb by skeletal muscle. Flow estimates were made serially as a function of variations in plasma glucose and insulin and changing the muscle contractile state by electrical stimulation. Flow ranged from 3.1 ml/min/100 g at rest to 71 ml/min/100 g during stimulation. There was good agreement between the two methods of flow measurement over the entire range of flows (r = 0.96 at a slope of 0.90). Flow measured by either method did not vary significantly from baseline over a range of plasma glucose from 5 to 30 mM and plasma insulin from 0 to 20 microU/ml. When flow was increased up to 20-fold by electrical stimulation there was a decrease in extraction of 82 Rb proportional to the increase in flow. However, at pharmacologic levels of insulin (greater than 150 microU/ml) flow was increased twofold as measured by radiolabeled microspheres, but not as measured by rubidium. There was no apparent decrease in extraction of 82 Rb with high insulin. The discrepancy between the microsphere measured flow and rubidium measured flow with high plasma insulin levels can be explained by the assumption that the expected decrease in the extraction fraction was counteracted by an increase in Na+/K+-ATPase activity. It is concluded that the first-pass flow model gives valid estimates of skeletal muscle blood flow in vivo with 82 Rb, provided that plasma insulin levels are normal

The valence and Rydberg states of difluoromethane: A combined experimental vacuum ultraviolet spectrum absorption and theoretical study by ab initio configuration interaction and density functional computations

Science.gov (United States)

Palmer, Michael H.; Vrønning Hoffmann, Søren; Jones, Nykola C.; Coreno, Marcello; de Simone, Monica; Grazioli, Cesare

2018-06-01

The vacuum ultraviolet (VUV) spectrum for CH2F2 from a new synchrotron study has been combined with earlier data and subjected to detailed scrutiny. The onset of absorption, band I and also band IV, is resolved into broad vibrational peaks, which contrast with the continuous absorption previously claimed. A new theoretical analysis, using a combination of time dependent density functional theory (TDDFT) calculations and complete active space self-consistent field, leads to a major new interpretation. Adiabatic excitation energies (AEEs) and vertical excitation energies, evaluated by these methods, are used to interpret the spectra in unprecedented detail using theoretical vibronic analysis. This includes both Franck-Condon (FC) and Herzberg-Teller (HT) effects on cold and hot bands. These results lead to the re-assignment of several known excited states and the identification of new ones. The lowest calculated AEE sequence for singlet states is 11B1 ˜ 11A2 expected; the onset of the 15.5 eV band shows a set of vibrational peaks, but the vibration frequency does not correspond to any of the photoelectron spectral (PES) structure and is clearly valence in nature. The routine use of PES footprints to detect Rydberg states in VUV spectra is shown to be inadequate. The combined effects of FC and HT in the VUV spectral bands lead to additional vibrations when compared with the PES.

Second CERN group produces cold atoms of antihydrogen

CERN Document Server

Levi-Goss, Barbara

2003-01-01

A new experiment, by CERN's ATRAP collaboration, which introduced a technique for determining the quantum state in which antihydrogen atoms are formed was discussed. To make antihydrogen, antiprotons were taken from CERN's Antiproton Decelerator, further slowed down, and trapped with a configuration of electric fields. The evidence gathered confirmed that the H over bar atoms formed in the experiment occupy highly excited Rydberg states. (Edited abstract) 5 Refs.

Crystal structure of ammonium and rubidium octacyanomolybdates (4)

Energy Technology Data Exchange (ETDEWEB)

Semenishin, D.I.; Glovyak, T.; Mys' kiv, M.G.

1985-01-01

By the method of monocrystal at the automatic diffractometer ''Syntex P2/sub 1/'' the crystal structure of ammonium and rubidium octacyanomolybdates (4)-(NH/sub 4/)/sub 4/(Mo(CN)/sub 8/)x0.5H/sub 2/O (1) (sp.gr. Pma5 2, a=15.50(3), b=14.118 (3), c=7.438 (1)A, Z=4, R=0.062 and Rb/sub 4/(Mo(CN)/sub 8/):3H/sub 2/O (2) (sp.gr. P4/sub 1/2/sub 1/2, a=9.300 (1), c=21.807 (3) A, Z=4, R=0.065) is determined. Mo atoms in the structure 1 occupy two 2(b) and 2(c) particular positions and are surrounded, each of them, by light CN-ligands. The mean values of Mo-C distances for Mo(1) are equal 2.216, for Mo(2)-2.235 A. Mo-N mean values, practically are identical in both molybdenum anions and are equal 3.353 A. MoCN angles are varied from 175.0 to 178.4. The dodecahedron with the only symmetry axis 2 corresponds to the Mo(1) coordination sphere whereas the Mo(2) atoms coordination polyhedron (CP) is the symmetry in antiprism. In the structure 2 Mo-C distances are in the limits of 2.130-2.160 and Mo-N 3.290-3.307 A. MoCN angles are varied from 176.0 to 179.3 deg, the (MoC/sub 8/) CP represents a symmetry 2 dodecahedron. The existence of two Mo coordination forms in the structure 1 is up to now the only example among structurally studied octacyanomolybdates (4).

Interference effects at photoionization of Rydberg atoms by a strong electromagnetic field

International Nuclear Information System (INIS)

Movsesyan, A.M.; Fedorov, M.V.

1989-01-01

The photoionization of Rydberg atoms in a strong electromagnetic field is considered. Degeneration of the levels with respect to the orbital moment, their Stark splitting and the possibility of resonant interaction with levels of lower energy are taken into account. The complex quasi-energies of the system, photoelectron spectrum in the limit of an infinite duration of interaction and the time dependence of the total ionization probability are found. It is shown that a narrowing of the quasi-energy levels occurs in a strong field. Against a background of the quasi- continuum the quasi-energy spectrum consists of more or less narrow levels. In this case the photoelectron spectrum acquires a multi-peak form. With increasing field strength the height of the peaks increases, whereas their width decreases. The ionization rate decreases with increasing field strength. The presence of a quasi-continuum is the cause of the partially non-exponential nature of the atomic disintegration

Absolute high-resolution Se+ photoionization cross-section measurements with Rydberg-series analysis

International Nuclear Information System (INIS)

Esteves, D. A.; Bilodeau, R. C.; Sterling, N. C.; Phaneuf, R. A.; Kilcoyne, A. L. D.; Red, E. C.; Aguilar, A.

2011-01-01

Absolute single photoionization cross-section measurements for Se + ions were performed at the Advanced Light Source (ALS) at Lawrence Berkeley National Laboratory using the photo-ion merged-beams technique. Measurements were made at a photon energy resolution of 5.5 meV from 17.75 to 21.85 eV spanning the 4s 2 4p 3 4 S 3/2 o ground-state ionization threshold and the 2 P 3/2 o , 2 P 1/2 o , 2 D 5/2 o , and 2 D 3/2 o metastable state thresholds. Extensive analysis of the complex resonant structure in this region identified numerous Rydberg series of resonances and obtained the Se 2+ 4s 2 4p 23 P 2 and 4s 2 4p 21 S 0 state energies. In addition, particular attention was given to removing significant effects in the measurements due to a small percentage of higher-order undulator radiation.

Comparison of the target-thickness dependence of the convoy electron yield and the Rydberg electron yield measured in coincidence with exit charge states in fast ion-solid collisions

International Nuclear Information System (INIS)

Gaither, C.C. III; Breinig, M.; Freyou, J.; Underwood, T.A.

1988-01-01

We have simultaneously measured the yield of convoy electrons and the yield of electrons in high Rydberg states of the projectile (n /approx gt/ 70), produced by 2MeV/u C projectiles passing through C foils, whose thicknesses range from 4--10 ug/cm 2 , for incident charge states q/sub i/ = 4--6 and exit charge states q/sub e/ = 4--6. We have found that these yields exhibit similar trends as a function of foil thickness, but that, nevertheless, the ratio of the number of convoy electrons detected in coincidence with ions of exit charge state q/sub e/ to the number of electrons detected in high Rydberg states of ions with the same exit charge state is a function of foil thickness. This may be due to a broadening of the convoy electron energy spectrum with increasing foil thickness. 6 refs., 3 figs

Cold injuries.

Science.gov (United States)

Kruse, R J

1995-01-01

There are two categories of cold injury. The first is hypothermia, which is a systemic injury to cold, and the second is frostbite, which is a local injury. Throughout history, entire armies, from George Washington to the Germans on the Russian Front in World War II, have fallen prey to prolonged cold exposure. Cold injury is common and can occur in all seasons if ambient temperature is lower than the core body temperature. In the 1985 Boston Marathon, even though it was 76 degrees and sunny, there were 75 runners treated for hypothermia. In general, humans adapt poorly to cold exposure. Children are at particular risk because of their relatively greater surface area/body mass ratio, causing them to cool even more rapidly than adults. Because of this, the human's best defense against cold injury is to limit his/her exposure to cold and to dress appropriately. If cold injury has occurred and is mild, often simple passive rewarming such as dry blankets and a warm room are sufficient treatment.

Deutsch, Toffoli, and cnot Gates via Rydberg Blockade of Neutral Atoms

Science.gov (United States)

Shi, Xiao-Feng

2018-05-01

Universal quantum gates and quantum error correction (QEC) lie at the heart of quantum-information science. Large-scale quantum computing depends on a universal set of quantum gates, in which some gates may be easily carried out, while others are restricted to certain physical systems. There is a unique three-qubit quantum gate called the Deutsch gate [D (θ )], from which a circuit can be constructed so that any feasible quantum computing is attainable. We design an easily realizable D (θ ) by using the Rydberg blockade of neutral atoms, where θ can be tuned to any value in [0 ,π ] by adjusting the strengths of external control fields. Using similar protocols, we further show that both the Toffoli and controlled-not gates can be achieved with only three laser pulses. The Toffoli gate, being universal for classical reversible computing, is also useful for QEC, which plays an important role in quantum communication and fault-tolerant quantum computation. The possibility and speed of realizing these gates shed light on the study of quantum information with neutral atoms.

The Excitation of Rydberg Atoms of Thallium in an Electric Field

Science.gov (United States)

Bokhan, P. A.; Zakrevskii, D. E.; Kim, V. A.; Fateev, N. V.

2018-01-01

The spectrum of excitation of Rydberg states of thallium atoms has been investigated using a collimated atomic beam in a two-step isotope selective laser scheme 62 P 1/2 → 62 D 3/2 → Tl** in the presence of an electric field with a strength of up to 1.5 kV/cm near the level 16 F 5/2. The optical transitions 6 D 3/2 → 18 D 3/2 and 6 D 3/2 → 16 G 7/2, which were induced by an external electric field and dipole-forbidden, have been studied experimentally. The values for the scalar polarizabilities (in units cm-1/(kV/cm)2) α0(16 F 5/2) = 3.71 ± 0.3, α0(18 D 3/2) = 11.70 ± 0.25, and α0(16 G 7/2) = 44.1 ± 0.9, which are compared with the calculated one, have been obtained. The new values of energy parameters for the states 18 D 3/2 and 16 G 7/2 have been determined.

Light in Condensed Matter in the Upper Atmosphere as the Origin of Homochirality: Circularly Polarized Light from Rydberg Matter

Science.gov (United States)

Holmlid, Leif

2009-08-01

Clouds of the condensed excited Rydberg matter (RM) exist in the atmospheres of comets and planetary bodies (most easily observed at Mercury and the Moon), where they surround the entire bodies. Vast such clouds are recently proposed to exist in the upper atmosphere of Earth (giving rise to the enormous features called noctilucent clouds, polar mesospheric clouds, and polar mesospheric summer radar echoes). It has been shown in experiments with RM that linearly polarized visible light scattered from an RM layer is transformed to circularly polarized light with a probability of approximately 50%. The circular Rydberg electrons in the magnetic field in the RM may be chiral scatterers. The magnetic and anisotropic RM medium acts as a circular polarizer probably by delaying one of the perpendicular components of the light wave. The delay process involved is called Rabi-flopping and gives delays of the order of femtoseconds. This strong effect thus gives intense circularly polarized visible and UV light within RM clouds. Amino acids and other chiral molecules will experience a strong interaction with this light field in the upper atmospheres of planets. The interaction will vary with the stereogenic conformation of the molecules and in all probability promote the survival of one enantiomer. Here, this strong effect is proposed to be the origin of homochirality. The formation of amino acids in the RM clouds is probably facilitated by the catalytic effect of RM.

Light in condensed matter in the upper atmosphere as the origin of homochirality: circularly polarized light from Rydberg matter.

Science.gov (United States)

Holmlid, Leif

2009-01-01

Clouds of the condensed excited Rydberg matter (RM) exist in the atmospheres of comets and planetary bodies (most easily observed at Mercury and the Moon), where they surround the entire bodies. Vast such clouds are recently proposed to exist in the upper atmosphere of Earth (giving rise to the enormous features called noctilucent clouds, polar mesospheric clouds, and polar mesospheric summer radar echoes). It has been shown in experiments with RM that linearly polarized visible light scattered from an RM layer is transformed to circularly polarized light with a probability of approximately 50%. The circular Rydberg electrons in the magnetic field in the RM may be chiral scatterers. The magnetic and anisotropic RM medium acts as a circular polarizer probably by delaying one of the perpendicular components of the light wave. The delay process involved is called Rabi-flopping and gives delays of the order of femtoseconds. This strong effect thus gives intense circularly polarized visible and UV light within RM clouds. Amino acids and other chiral molecules will experience a strong interaction with this light field in the upper atmospheres of planets. The interaction will vary with the stereogenic conformation of the molecules and in all probability promote the survival of one enantiomer. Here, this strong effect is proposed to be the origin of homochirality. The formation of amino acids in the RM clouds is probably facilitated by the catalytic effect of RM.

AEgIS experiment: Towards antihydrogen beam production for antimatter gravity measurements

CERN Document Server

Mariazzi, Sebastiano; Amsler, Claude; Ariga, Akitaka; Ariga, Tomoko; Belov, Alexandre S; Bonomi, Germano; Bräunig, Philippe; Brusa, Roberto S; Bremer, Johan; Cabaret, Louis; Canali, Carlo; Caravita, Ruggero; Castelli, Fabrizio; Cerchiari, Giovanni; Cialdi, Simone; Comparat, Daniel; Consolati, Giovanni; Dassa, Luca; Derking, Jan Hendrik; Di Domizio, Sergio; Di Noto, Lea; Doser, Michael; Dudarev, Alexey; Ereditato, Antonio; Ferragut, Rafael; Fontana, Andrea; Genova, Pablo; Giammarchi, Marco; Gligorova, Angela; Gninenko, Sergei N; Hogan, Stephen D; Haider, Stefan; Jordan, Elena; Jørgensen, Lars V; Kaltenbacher, Thomas; Kawada, Jiro; Kellerbauer, Alban; Kimura, Mitsuhiro; Knecht, Andreas; Krasnický, Daniel; Lagomarsino, Vittorio; Lehner, Sebastian; Malbrunot, Chloe; Matveev, Viktor A; Merkt, Frederic; Moia, Fabio; Nebbia, Giancarlo; Nédélec, Patrick; Oberthaler, Markus K; Pacifico, Nicola; Petráček, Vojtech; Pistillo, Ciro; Prelz, Francesco; Prevedelli, Marco; Regenfus, Christian; Riccardi, Cristina; Røhne, Ole; Rotondi, Alberto; Sandaker, Heidi; Scampoli, Paola; Storey, James; Subieta Vasquez, Martin A.; Spaček, Michal; Czech Technical U. in Prague - FNSPE - B\\oehova 7 - 11519 - Praha 1 - Czech Aff25 Testera, Gemma; Vaccarone, Renzo; Villa, Fabio; Widmann, Eberhard; Zavatarelli, Sandra; Zmeskal, Johann

2014-01-01

AEgIS (Antimatter Experiment: Gravity, Interferometry, Spectroscopy) is an experiment that aims to perform the first direct measurement of the gravitational acceleration g of antihydrogen in the Earth’s field. A cold antihydrogen beam will be produced by charge exchange reaction between cold antiprotons and positronium excited in Rydberg states. Rydberg positronium (with quantum number n between 20 and 30) will be produced by a two steps laser excitation. The antihydrogen beam, after being accelerated by Stark effect, will fly through the gratings of a moir ́ e deflectometer. The deflection of the horizontal beam due to its free fall will be measured by a position sensitive detector. It is estimated that the detection of about 10 3 antihydrogen atoms is required to determine the gravitational acceleration with a precision of 1%. In this report an overview of the AEgIS experiment is presented and its current status is described. Details on the production of slow positronium and its excitation with lasers ar...

Temporal Bell-type inequalities for two-level Rydberg atoms coupled to a high-Q resonator

International Nuclear Information System (INIS)

Huelga, S.F.; Marshall, T.W.; Santos, E.

1996-01-01

Following the strategy of showing specific quantum effects by means of the violation of a classical inequality, a pair of Bell-type inequalities is derived on the basis of certain additional assumptions, whose plausibility is discussed in detail. Such inequalities are violated by the quantum mechanical predictions for the interaction of a two-level Rydberg atom with a single mode sustained by a high-Q resonator. The experimental conditions required in order to show the existence of forbidden values, according to a hidden variables formalism, in a real experiment are analyzed for various initial field statistics. In particular, the revival dynamics expected for the interaction with a coherent field leads to classically forbidden values, which would indicate a purely quantum effect. copyright 1996 The American Physical Society

A study on the performance of an electrostatic focusing mirror for Rydberg positronium

Science.gov (United States)

Jones, Adric C. L.; Cecchini, Gabriel G.; Moxom, Jeremy; Osorno, Kevin; Rutbeck-Goldman, Harris J.; Fuentes-Garcia, Melina; Greaves, Rod G.; Adams, Daniel J.; Tom, Harry W. K.; Mills, Allen P., Jr.

2018-01-01

Recently, we demonstrated an electrostatic mirror that focuses a beam of Rydberg positronium atoms over a 6 m path to a 32 ± 1 mm FWHM diameter spot on a position sensitive detector. The mirror is comprised of 360 wires arranged in the shape of a nearly-cylindrical revolved truncated ellipse 96 mm in radius, with potentials of equal and opposite magnitude applied to alternating wires to create a short-ranged electric field that decreases in magnitude exponentially with e-folding length = 0.53 mm. Here, we explore in detail the observed resolution and discuss the factors contributing to its broadening from the ideal point focus of a perfect embodiment of the mirror. Improvements to the design are considered, with the aim to achieve a mirror with a resolution of <0.5 mm, which is necessary for a proposed measurement of the gravitational deflection of positronium.

Spin-polarized hydrogen Rydberg time-of-flight: Experimental measurement of the velocity-dependent H atom spin-polarization

International Nuclear Information System (INIS)

Broderick, Bernadette M.; Lee, Yumin; Doyle, Michael B.; Chernyak, Vladimir Y.; Suits, Arthur G.; Vasyutinskii, Oleg S.

2014-01-01

We have developed a new experimental method allowing direct detection of the velocity dependent spin-polarization of hydrogen atoms produced in photodissociation. The technique, which is a variation on the H atom Rydberg time-of-flight method, employs a double-resonance excitation scheme and experimental geometry that yields the two coherent orientation parameters as a function of recoil speed for scattering perpendicular to the laser propagation direction. The approach, apparatus, and optical layout we employ are described here in detail and demonstrated in application to HBr and DBr photolysis at 213 nm. We also discuss the theoretical foundation for the approach, as well as the resolution and sensitivity we achieve

Cold plate

Energy Technology Data Exchange (ETDEWEB)

Marroquin, Christopher M.; O' Connell, Kevin M.; Schultz, Mark D.; Tian, Shurong

2018-02-13

A cold plate, an electronic assembly including a cold plate, and a method for forming a cold plate are provided. The cold plate includes an interface plate and an opposing plate that form a plenum. The cold plate includes a plurality of active areas arranged for alignment over respective heat generating portions of an electronic assembly, and non-active areas between the active areas. A cooling fluid flows through the plenum. The plenum, at the non-active areas, has a reduced width and/or reduced height relative to the plenum at the active areas. The reduced width and/or height of the plenum, and exterior dimensions of cold plate, at the non-active areas allow the non-active areas to flex to accommodate surface variations of the electronics assembly. The reduced width and/or height non-active areas can be specifically shaped to fit between physical features of the electronics assembly.

Excitation of helium Rydberg states and doubly excited resonances in strong extreme ultraviolet fields: Full-dimensional quantum dynamics using exponentially tempered Gaussian basis sets

Czech Academy of Sciences Publication Activity Database

Kaprálová-Žďánská, Petra Ruth; Šmydke, Jan; Civiš, S.

2013-01-01

Roč. 139, č. 10 (2013), s. 104314 ISSN 0021-9606 R&D Projects: GA AV ČR IAAX00100903; GA MŠk(CZ) ME10046; GA ČR GAP205/11/0571 Institutional support: RVO:68378271 Keywords : Gaussian distribution * helium * oscillator strengths * quantum chemistry * rotational states * Rydberg states * two-photon processes Subject RIV: BL - Plasma and Gas Discharge Physics Impact factor: 3.122, year: 2013

Myocardial perfusion of infarcted and normal myocardium in propofol-anesthetized minipigs using ⁸²Rubidium PET

DEFF Research Database (Denmark)

Rasmussen, Thomas; Larsen, Bjarke Follin; Kastrup, Jens

2016-01-01

Cardiac Rubidium-82 (82Rb) positron-emission-tomography (PET) is a good method for quantification of myocardial blood flow in man. Quantification of myocardial blood flow in animals to evaluate new treatment strategies or to understand underlying disease is also of great interest but raises some...... challenges. Animals, which have been anesthetized during PET acquisition, might react differently to used stress medications, and therefore difficulties might exist while evaluating the resulting PET images using standard software packages from commercial vendors optimized for human hearts. Furthermore...... propofol, used for anesthesia, can influence myocardial perfusion and coronary flow reserve due to its vasorelaxant effect, and interactions might exist between propofol and used stress agents, potentially affecting the result of the examination. We present cardiac 82Rb-PET studies performed in propofol...

Low-energy experiments that measure fundamental constants and test basic symmetries

CERN Multimedia

CERN. Geneva. Audiovisual Unit

2002-01-01

Cold Antihydrogen: Are We There? Cold antihydrogen offers the possibility to precisely compare the structure of antihydrogen and hydrogen atoms, using the well developed tools of laser spectroscopy with antihydrogen atoms cold enough to be trapped in the minimum of a magnetic field gradient. Progress made at CERN's new Antiproton Decelerator will be discussed, along with goals and aspirations, such as measuring the anti-Rydberg constant. ATRAP has observed and studied the interaction of low energy antiprotons and positrons for more than a year, and ATHENA hopes to soon make antiprotons and positrons to interact as well.

Interaction of Rydberg atoms with two contrapropagating ultrashort laser pulses

International Nuclear Information System (INIS)

Lugovskoy, A. V.; Bray, I.

2006-01-01

In this paper we investigate how Rydberg atoms respond to perturbation by two contrapropagating ultrashort laser pulses. We consider the case where the durations of both pulses τ 1 and τ 2 are shorter than the inverse of the initial-state energy ε i -1 . When acting alone such a pulse passes through the atom without noticeable alteration in the atomic state. The situation is different if two such pulses interfere in the region of atom localization. In this case the atomic response is significantly enhanced. This is due to the nonzero momentum transferred to the electron by the interplay of the electric field of one pulse and the magnetic field of the other. The sudden perturbation approximation is used to evaluate the transition probabilities. They are shown to depend on the atom position with respect to the pulse interference region. This dependence is determined by the relationship between the atomic diameter d i and the interference-region size l=c(τ 1 +τ 2 ) (c is the speed of light). If d i i >>l the transition probabilities are sensitive to the electron density distribution along the propagation direction. The probabilities of the initial-state destruction and atom ionization drop as l/d i irrespective of the characteristics of the pulses

Conceptualizing Cold Disasters

DEFF Research Database (Denmark)

Lauta, Kristian Cedervall; Dahlberg, Rasmus; Vendelø, Morten Thanning

2017-01-01

In the present article, we explore in more depth the particular circumstances and characteristics of governing what we call ‘cold disasters’, and thereby, the paper sets out to investigate how disasters in cold contexts distinguish themselves from other disasters, and what the implications hereof...... are for the conceptualization and governance of cold disasters. Hence, the paper can also be viewed as a response to Alexander’s (2012a) recent call for new theory in the field of disaster risk reduction. The article is structured in four overall parts. The first part, Cold Context, provides an overview of the specific...... conditions in a cold context, exemplified by the Arctic, and zooms in on Greenland to provide more specific background for the paper. The second part, Disasters in Cold Contexts, discusses “cold disasters” in relation to disaster theory, in order to, elucidate how cold disasters challenge existing...

Promotion of radiation peroxidation in models of lipid membranes by caesium and rubidium counter-ions: micellar linolenic acids

Energy Technology Data Exchange (ETDEWEB)

Raleigh, J A; Kremers, W [Atomic Energy of Canada Ltd., Pinawa, Manitoba. Whiteshell Nuclear Research Establishment

1978-11-01

Caesium and rubidium counter-ions increase peroxidation in irradiated micelles of linoleic (18 : 2) and linolenic (18 :3) acids. The effect was specific to Cs/sup +/ and Rb/sup +/ in the alkali metal series. The effect was independent of the salts used (Cl/sup -/, NO/sub 3//sup -/, Cl0/sub 4//sup -/) and, therefore, independent of the chaotropic nature, and reactivity with hydroxyl radicals of Cl/sup -/, NO/sub 3//sup -/ and ClO/sub 4//sup -/. The promotion of peroxidation by Cs/sup +/ and Rb/sup +/ is interpreted in terms of their effect on fatty acid micelle structure. The dependence of radiation peroxidation on lipid structure in the micelles may be significant for studies of peroxidation in highly structured cell membranes.

High-resolution measurements and multichannel quantum defect analysis of spectral line shapes of autoionizing Rydberg series

International Nuclear Information System (INIS)

Ueda, Kiyoshi

1997-01-01

Spectral line shapes for autoionizing Rydberg series are briefly reviewed within the framework of multichannel quantum defect theory (MQDT). Recent high-resolution measurements and MQDT analysis for the spectra line shapes are reviewed for the mp 5 ( 2 P 1/2 )ns ' and nd ' J=1 odd spectra of the Ar, Kr, and Xe atoms (m=3,4,5 for Ar, Kr, and Xe) and the 3p 5 ( 2 P 1/2 )nd ' J=2 and 3 odd spectra of Ar*3p 5 4p excited atoms. Some results are also discussed for the Ca 4p( 2 P 1/2,3/2 )ns and nd J=1 odd spectrum and the Ba 5d( 2 P 5/2 )nd J=1 odd spectrum

Vapor cell geometry effect on Rydberg atom-based microwave electric field measurement

Science.gov (United States)

Zhang, Linjie; Liu, Jiasheng; Jia, Yue; Zhang, Hao; Song, Zhenfei; Jia, Suotang

2018-03-01

The geometry effect of a vapor cell on the metrology of a microwave electric field is investigated. Based on the splitting of the electromagnetically induced transparency spectra of cesium Rydberg atoms in a vapor cell, high-resolution spatial distribution of the microwave electric field strength is achieved for both a cubic cell and a cylinder cell. The spatial distribution of the microwave field strength in two dimensions is measured with sub-wavelength resolution. The experimental results show that the shape of a vapor cell has a significant influence on the abnormal spatial distribution because of the Fabry–Pérot effect inside a vapor cell. A theoretical simulation is obtained for different vapor cell wall thicknesses and shows that a restricted wall thickness results in a measurement fluctuation smaller than 3% at the center of the vapor cell. Project supported by the National Key Research and Development Program of China (Grant Nos. 2017YFA03044200 and 2016YFF0200104), the National Natural Science Foundation of China (Grant Nos. 91536110, 61505099, and 61378013), and the Fund for Shanxi “331 Project” Key Subjects Construction, China.

Mineralogy of the fraction and age estimation rubidium - strontium of the Bambui Group, MG, Brazil

International Nuclear Information System (INIS)

Bonhomme, M.G.

1976-01-01

A study of the illite crystallinity of sediments of the Upper Precambrian Bambui Group, MG, has been done to determine the zones without metamorphism, the only ones able to give the age of the sedimentation. Only the region of Januaria escaped from any sensible thermo-tectonic event. The Bambui sediments contain well crystallized vermiculite probably formed during the anchimetamorphism. The rubidium-strontium age obtained in Januaria (619 + - 17 m.y.) corresponds in fact to the main phase of the Brazilian orogenic cycle. The late isotopic homogeneization was caused by a strong late diagenesis. The anchimetamorphic phosphateous sediments in Cedro do Abate show that the ferro-magnesian illite is a more easely open system than aluminous illite, and in this case dates the later event of the Brazilian cycle at 445 + - 25 m.y. The age of 600 m.y. for the metamorphism is a younger limit for the real age of the Bambui, the late Precambrian age of which is confirmed

EDITORIAL: Focus on Cold and Ultracold Molecules FOCUS ON COLD AND ULTRACOLD MOLECULES

Science.gov (United States)

Carr, Lincoln D.; Ye, Jun

2009-05-01

and H Pu Collisions of bosonic ultracold polar molecules in microwave traps Alexander V Avdeenkov Cold TiO(X3Δ)-He collisions Mei-Ju Lu and Jonathan D Weinstein Investigation of dephasing rates in an interacting Rydberg gas U Raitzsch, R Heidemann, H Weimer, B Butscher, P Kollmann, R Löw, H P Büchler and T Pfau Impact of electric fields on highly excited rovibrational states of polar dimers Rosario González-Férez and Peter Schmelcher Phase transition from straight into twisted vortex lines in dipolar Bose-Einstein condensates M Klawunn and L Santos Stimulating the production of deeply bound RbCs molecules with laser pulses: the role of spin-orbit coupling in forming ultracold molecules Subhas Ghosal, Richard J Doyle, Christiane P Koch and Jeremy M Hutson Sensitive measurement of mp/me variance using vibrational transition frequencies of cold molecules Masatoshi Kajita

Cold urticaria. Dissociation of cold-evoked histamine release and urticara following cold challenge.

Science.gov (United States)

Keahey, T M; Greaves, M W

1980-02-01

Nine patients with acquired cold urticaria were studied to assess the effects of beta-adrenergic agents, xanthines, and corticosteroids on cold-evoked histamine release from skin in vivo. The patients, in all of whom an immediate urticarial response developed after cooling of the forearm, demonstrated release of histamine into the venous blood draining that forearm. Following treatment with aminophylline and albuterol in combination or prednisone alone, suppression of histamine release occurred in all but one patient. In some patients, this was accompanied by a subjective diminution in pruritus or buring, but there was no significant improvement in the ensuing edema or erythema. In one patient, total suppression of histamine release was achieved without any effect on whealing and erythema in response to cold challenge. Our results suggest that histamine is not central to the pathogenesis of vascular changes in acquired cold urticaria.

Coherent states of the driven Rydberg atom: Quantum-classical correspondence of periodically driven systems

International Nuclear Information System (INIS)

Vela-Arevalo, Luz V.; Fox, Ronald F.

2005-01-01

A methodology to calculate generalized coherent states for a periodically driven system is presented. We study wave packets constructed as a linear combination of suitable Floquet states of the three-dimensional Rydberg atom in a microwave field. The driven coherent states show classical space localization, spreading, and revivals and remain localized along the classical trajectory. The microwave strength and frequency have a great effect in the localization of Floquet states, since quasienergy avoided crossings produce delocalization of the Floquet states, showing that tuning of the parameters is very important. Using wavelet-based time-frequency analysis, the classical phase-space structure is determined, which allows us to show that the driven coherent state is located in a large regular region in which the z coordinate is in resonance with the external field. The expectation values of the wave packet show that the driven coherent state evolves along the classical trajectory

Matterwave interferometric velocimetry of cold Rb atoms

Science.gov (United States)

Carey, Max; Belal, Mohammad; Himsworth, Matthew; Bateman, James; Freegarde, Tim

2018-03-01

We consider the matterwave interferometric measurement of atomic velocities, which forms a building block for all matterwave inertial measurements. A theoretical analysis, addressing both the laboratory and atomic frames and accounting for residual Doppler sensitivity in the beamsplitter and recombiner pulses, is followed by an experimental demonstration, with measurements of the velocity distribution within a 20 ?K cloud of rubidium atoms. Our experiments use Raman transitions between the long-lived ground hyperfine states, and allow quadrature measurements that yield the full complex interferometer signal and hence discriminate between positive and negative velocities. The technique is most suitable for measurement of colder samples.

Summary of theory and techniques, sample selection and project organization for potassium-argon, rubidium-strontium and fission track dating and strontium isotope studies

International Nuclear Information System (INIS)

Adams, C.J.; Graham, I.J.; Seward, D.

1987-02-01

A brief outline is given of the theory and techniques of the potassium-argon, rubidium-strontium and fission-track dating methods and related isotope studies which are currently in use at the Institute of Nuclear Sciences, DSIR. Some limitations of each technique are set out in terms of age range and materials for dating, and the appropriate choice of various mineral and rock types and subsequent age interpretations are discussed. The organisation of project proposals and categories is described and procedures for sample submission and documentation are given

Effect of optical pumping on absorption spectra for the doppler broadened rubidium

International Nuclear Information System (INIS)

Shin, Seo Ro; Noh, Heung Ryoul

2008-01-01

The absorption of a laser beam in the Doppler broadened atomic vapor cell is one of the simplest problems in atomic physics. Although many reports on theoretical and experimental studies of linear absorption have been reported, the effect of optical pumping on the absorption coefficient has not been studied in detail. In this presentation, we present a theoretical and experimental study on linear absorption for the Doppler broadened rubidium vapor cell. The absorption coefficient of a σ"+"(or π)polarized laser beam was calculated as a function of the laser frequency for the various laser intensities. The calculated results were compared with the experimental results. Figure 1(a) shows the calculated absorption coefficient of the π polarized laser beam for the transition F"g"=1→F"e"=0,1,2 of the "87"Rb atom. The diameter of the laser beam was 3mm and the intensity was I=0 and I=0.1I"8"(I"8"=16.2W/m"2"). The peak values for various intensities are shown in Fig. 1(b). We found that the absorption coefficient for the transition from the lower hyperfine state decreased with the increased laser intensity, whereas that for the transition from the upper hyperfine state increased(decreased)for the σ"+"(π)polarized laser beam

Rubidium-strontium chronology of the metamorphism and prehistory of central Australian granulites

Energy Technology Data Exchange (ETDEWEB)

Gray, C M [La Trobe Univ., Bundoora (Australia); Compston, W

1978-11-01

Rubidium-strontium isotopic study of intermediate-pressure granulites at Mt. Aloysius, central Australia reveals total rock isochrons that either record the metamorphism or predate it. The gneisses involved, typically quartz + feldspar + orthopyroxene + garnet granulites, occur in five lithological units which outline a simple fold structure. The distribution of isotopic ages in a 25 km/sup 2/ area is tested using 74 samples collected in groups of 2 to 4 both along and across strike in each of the units. Two total rock isochron ages of 1200 and 1550 Myr occur, and both are found at different sites in one unit. Mineral ages are younger and independent of location, with feldspars giving 800 Myr and biotites 730 Myr. The 1200 Myr isochrons show the features of outcrop-scale Sr isotopic homogenisation and are taken to record the time of metamorphism. Contemporaneous regional depletion of U, commonly associated with granulite facies metamorphism, confirms the interpretation. The 1550 Myr isochrons describe entire lithological units and are best assigned to the supracrustal genesis of the rocks. The preservation of two ages indicates that isotopic equilibration of anhydrous total rocks is incomplete even within the granulite facies. Careful interpretation is required to assign geological meaning to granulite isochrons.

Relationships of self-identified cold tolerance and cold-induced vasodilatation in the finger

Science.gov (United States)

Park, Joonhee; Lee, Joo-Young

2016-04-01

This study was conducted to investigate relationships of self-identified cold tolerance and cold-induced vasodilatation (CIVD) in the finger. Nine males and 34 females participated in the following 2 tests: a CIVD test and a self-reported survey. The CIVD test was conducted 30-min cold-water immersion (3.8 ± 0.3 °C) of the middle finger at an air temperature of 27.9 ± 0.1 °C. The self-reported questionnaire consisted of 28 questions about whole and local body cold and heat tolerances. By a cluster analysis on the survey results, the participants were divided into two groups: high self-identified cold tolerance (HSCT, n = 25) and low self-identified cold tolerance (LSCT, n = 18). LSCT had lower self-identified cold tolerance ( P cold or heat tolerance had relationships with cold tolerance index, T max, and amplitude ( P cold tolerance classified through a standardized survey could be a good index to predict physiological cold tolerance.

Fractional Stark state selective electric field ionization of very high-n Rydberg states of molecules

International Nuclear Information System (INIS)

Dietrich, H.; Mueller-Dethlefs, K.; Baranov, L.Y.

1996-01-01

For the first time fractional Stark state selective electric field ionization of very high-n (n approx-gt 250) molecular Rydberg states is observed. An open-quote open-quote offset close-quote close-quote electric pulse selectively ionizes the more fragile open-quote open-quote red close-quote close-quote (down shifted in energy) Stark states. The more resilient open-quote open-quote bluer close-quote close-quote, or up-shifted, ones survive and are shifted down in energy upon application of a second (open-quote open-quote probe close-quote close-quote) pulse of opposite direction (diabatic Stark states close-quote inversion). Hence, even for smaller probe than offset fields ionization is observed. The offset/probe ratio allows one to control spectral peak shapes in zero-kinetic-energy photoelectron spectroscopy. copyright 1995 The American Physical Society

Burning Cold: Involvement of TRPA1 in Noxious Cold Sensation

OpenAIRE

Kwan, Kelvin Y.; Corey, David P.

2009-01-01

Soon after its discovery ten years ago, the ion channel TRPA1 was proposed as a sensor of noxious cold. Evidence for its activation by painfully cold temperatures (below ~15° C) has been mixed, however. Some groups found that cold elicits a nonselective conductance in cells expressing TRPA1; others found no activation, or argued that activation is an indirect effect of elevated \\(Ca^{ 2+}\\) . Sensory cells from the trigeminal and dorsal root ganglia that are activated by cold were sometimes c...

Cold-Hearted or Cool-Headed: Physical Coldness Promotes Utilitarian Moral Judgment

Directory of Open Access Journals (Sweden)

Hiroko eNakamura

2014-10-01

Full Text Available In the current study, we examine the effect of physical coldness on personal moral dilemma judgment. Previous studies have indicated that utilitarian moral judgment—sacrificing a few people to achieve the greater good for others—was facilitated when: (1 participants suppressed an initial emotional response and deliberately thought about the utility of outcomes; (2 participants had a high-level construal mindset and focused on abstract goals (e.g., save many; or (3 there was a decreasing emotional response to sacrificing a few. In two experiments, we exposed participants to extreme cold or typical room temperature and then asked them to make personal moral dilemma judgments. The results of Experiment 1 indicated that coldness prompted utilitarian judgment, but the effect of coldness was independent from deliberate thought or abstract high-level construal mindset. As Experiment 2 revealed, coldness facilitated utilitarian judgment via reduced empathic feelings. Therefore, physical coldness did not affect the cool-headed deliberate process or the abstract high-level construal mindset. Rather, coldness biased people toward being cold-hearted, reduced empathetic concern about a sacrificed victim, and facilitated utilitarian moral judgments.

Rubidium contents in erythrocyte of children, rice and soil in the areas with different selenium status

International Nuclear Information System (INIS)

Liu Nianqing; Zhao Shunying; Qian Qinfang; Zhu Lianzhen; Piao Jianhua

1997-01-01

Rubidium concentration of erythrocyte of healthy children aged from 6-11 years living in four areas of Sichuan Province with different selenium status was measured by PIXE and the results show that the Rb concentration in erythrocyte for the Keshan Disease area is two times more than other three areas. Meanwhile the glutathione peroxidase (GSHPx) activity of erythrocyte was determined and the results confirm that children in the Keshan Disease area are really with selenium deficiency. The Rb contents in rice and soil samples from the Keshan Disease area and the Se-deficiency area but with Se-supplementation to the inhabitants, were tested by INNA. It was found that Rb contents in rice and soil from the former area were much higher than those from the latter. This result indicates that Rb in erythrocyte of children is mainly taken from staple food (rice) and that a higher Rb level in soil is probably another environmental factor causing the Keshan Disease

Rydberg Atoms in Strong Fields: a Testing Ground for Quantum Chaos.

Science.gov (United States)

Courtney, Michael

1995-01-01

Rydberg atoms in strong static electric and magnetic fields provide experimentally accessible systems for studying the connections between classical chaos and quantum mechanics in the semiclassical limit. This experimental accessibility has motivated the development of reliable quantum mechanical solutions. This thesis uses both experimental and computed quantum spectra to test the central approaches to quantum chaos. These central approaches consist mainly of developing methods to compute the spectra of quantum systems in non -perturbative regimes, correlating statistical descriptions of eigenvalues with the classical behavior of the same Hamiltonian, and the development of semiclassical methods such as periodic-orbit theory. Particular emphasis is given to identifying the spectral signature of recurrences --quantum wave packets which follow classical orbits. The new findings include: the breakdown of the connection between energy-level statistics and classical chaos in odd-parity diamagnetic lithium, the discovery of the signature of very long period orbits in atomic spectra, quantitative evidence for the scattering of recurrences by the alkali -metal core, quantitative description of the behavior of recurrences near bifurcations, and a semiclassical interpretation of the evolution of continuum Stark spectra. (Copies available exclusively from MIT Libraries, Rm. 14-0551, Cambridge, MA 02139-4307. Ph. 617-253-5668; Fax 617-253-1690.).

Forward and backward scattering experiments in ultra-cold Rubidium atoms

DEFF Research Database (Denmark)

Kampel, Nir Shlomo

project, we have studied coherent forward scattering in the form of a memory experiment. In such an experiment we convert the input light pulse to an atomic excitation, and at a later time convert back the atomic excitation into the retrieved light pulse. In the first project, we investigate the source...

Grooved cold moderator tests

International Nuclear Information System (INIS)

Inoue, K.; Kiyanagi, Y.; Iwasa, H.; Watanabe, N.; Ikeda, S.; Carpenter, J.M.; Ishikawa, Y.

1983-01-01

We performed some grooved cold moderator experiments for methane at 20 K by using the Hokkaido University linac to obtain information to be used in the planning of the KENS-I' project. Cold neutron gains, spatial distribution of emitted beams and time distribution of the neutrons in the grooved cold moderator were measured. Furthermore, we assessed the effects of the grooved cold moderator on the performances of the spectrometers presently installed at the KENS-I cold source. We concluded that the grooved cold moderator benefited appreciably the performances of the spectrometers

Valence and lowest Rydberg electronic states of phenol investigated by synchrotron radiation and theoretical methods

Energy Technology Data Exchange (ETDEWEB)

Limão-Vieira, P., E-mail: plimaovieira@fct.unl.pt; Ferreira da Silva, F.; Lange, E. [Laboratório de Colisões Atómicas e Moleculares, CEFITEC, Departamento de Física, Faculdade de Ciências e Tecnologia, Universidade NOVA de Lisboa, 2829-516 Caparica (Portugal); Duflot, D. [Univ. Lille, UMR 8523–Physique des Lasers Atomes et Molécules, F-59000 Lille (France); CNRS, UMR 8523, F-59000 Lille (France); Jones, N. C.; Hoffmann, S. V. [ISA, Department of Physics and Astronomy, Aarhus University, Ny Munkegade 120, DK-8000 Aarhus C (Denmark); Śmiałek, M. A. [Department of Control and Power Engineering, Faculty of Ocean Engineering and Ship Technology, Gdańsk University of Technology, Gabriela Narutowicza 11/12, 80-233 Gdańsk (Poland); Department of Physical Sciences, The Open University, Walton Hall, MK7 6AA Milton Keynes (United Kingdom); Jones, D. B. [School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001 (Australia); Brunger, M. J. [School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001 (Australia); Institute of Mathematical Sciences, University of Malaya, 50603 Kuala Lumpur (Malaysia)

2016-07-21

We present the experimental high-resolution vacuum ultraviolet (VUV) photoabsorption spectra of phenol covering for the first time the full 4.3–10.8 eV energy-range, with absolute cross sections determined. Theoretical calculations on the vertical excitation energies and oscillator strengths were performed using time-dependent density functional theory and the equation-of-motion coupled cluster method restricted to single and double excitations level. These have been used in the assignment of valence and Rydberg transitions of the phenol molecule. The VUV spectrum reveals several new features not previously reported in the literature, with particular reference to the 6.401 eV transition, which is here assigned to the 3sσ/σ{sup ∗}(OH)←3π(3a″) transition. The measured absolute photoabsorption cross sections have been used to calculate the photolysis lifetime of phenol in the earth’s atmosphere (0–50 km).

Towards Quantum Simulation with Circular Rydberg Atoms

Directory of Open Access Journals (Sweden)

T. L. Nguyen

2018-02-01

Full Text Available The main objective of quantum simulation is an in-depth understanding of many-body physics, which is important for fundamental issues (quantum phase transitions, transport, … and for the development of innovative materials. Analytic approaches to many-body systems are limited, and the huge size of their Hilbert space makes numerical simulations on classical computers intractable. A quantum simulator avoids these limitations by transcribing the system of interest into another, with the same dynamics but with interaction parameters under control and with experimental access to all relevant observables. Quantum simulation of spin systems is being explored with trapped ions, neutral atoms, and superconducting devices. We propose here a new paradigm for quantum simulation of spin-1/2 arrays, providing unprecedented flexibility and allowing one to explore domains beyond the reach of other platforms. It is based on laser-trapped circular Rydberg atoms. Their long intrinsic lifetimes, combined with the inhibition of their microwave spontaneous emission and their low sensitivity to collisions and photoionization, make trapping lifetimes in the minute range realistic with state-of-the-art techniques. Ultracold defect-free circular atom chains can be prepared by a variant of the evaporative cooling method. This method also leads to the detection of arbitrary spin observables with single-site resolution. The proposed simulator realizes an XXZ spin-1/2 Hamiltonian with nearest-neighbor couplings ranging from a few to tens of kilohertz. All the model parameters can be dynamically tuned at will, making a large range of simulations accessible. The system evolution can be followed over times in the range of seconds, long enough to be relevant for ground-state adiabatic preparation and for the study of thermalization, disorder, or Floquet time crystals. The proposed platform already presents unrivaled features for quantum simulation of regular spin chains. We

Towards Quantum Simulation with Circular Rydberg Atoms

Science.gov (United States)

Nguyen, T. L.; Raimond, J. M.; Sayrin, C.; Cortiñas, R.; Cantat-Moltrecht, T.; Assemat, F.; Dotsenko, I.; Gleyzes, S.; Haroche, S.; Roux, G.; Jolicoeur, Th.; Brune, M.

2018-01-01

The main objective of quantum simulation is an in-depth understanding of many-body physics, which is important for fundamental issues (quantum phase transitions, transport, …) and for the development of innovative materials. Analytic approaches to many-body systems are limited, and the huge size of their Hilbert space makes numerical simulations on classical computers intractable. A quantum simulator avoids these limitations by transcribing the system of interest into another, with the same dynamics but with interaction parameters under control and with experimental access to all relevant observables. Quantum simulation of spin systems is being explored with trapped ions, neutral atoms, and superconducting devices. We propose here a new paradigm for quantum simulation of spin-1 /2 arrays, providing unprecedented flexibility and allowing one to explore domains beyond the reach of other platforms. It is based on laser-trapped circular Rydberg atoms. Their long intrinsic lifetimes, combined with the inhibition of their microwave spontaneous emission and their low sensitivity to collisions and photoionization, make trapping lifetimes in the minute range realistic with state-of-the-art techniques. Ultracold defect-free circular atom chains can be prepared by a variant of the evaporative cooling method. This method also leads to the detection of arbitrary spin observables with single-site resolution. The proposed simulator realizes an X X Z spin-1 /2 Hamiltonian with nearest-neighbor couplings ranging from a few to tens of kilohertz. All the model parameters can be dynamically tuned at will, making a large range of simulations accessible. The system evolution can be followed over times in the range of seconds, long enough to be relevant for ground-state adiabatic preparation and for the study of thermalization, disorder, or Floquet time crystals. The proposed platform already presents unrivaled features for quantum simulation of regular spin chains. We discuss

Cold acclimation increases cold tolerance independently of diapause programing in the bean bug, Riptortus pedestris.

Science.gov (United States)

Rozsypal, J; Moos, M; Goto, S G

2017-10-17

The bean bug (Riptortus pedestris) is a pest of soybeans and other legumes in Japan and other Asian countries. It enters a facultative adult diapause on exposure to short days. While photoperiodism and diapause are well understood in R. pedestris, knowledge of cold tolerance is very limited, as is information on the effect of diapause on cold tolerance. We examined the effect of photoperiod, cold acclimation, and feeding status on cold tolerance in R. pedestris. We found that cold acclimation significantly increased survival at -10°C in both long- and short-day adult R. pedestris. Since the difference in cold survival between long- and short-day cold-acclimated groups was only marginal, we conclude that entering diapause is not crucial for R. pedestris to successfully pass through cold acclimation and become cold tolerant. We observed similar effects in 5th instar nymphs, with both long- and short-day cold-acclimated groups surviving longer cold exposures compared with non-acclimated groups. Starvation, which was tested only in adult bugs, had only a negligible and negative impact on cold survival. Although cold tolerance significantly increased with cold acclimation in adult bugs, supercooling capacity unexpectedly decreased. Our results suggest that changes in supercooling capacity as well as in water content are unrelated to cold tolerance in R. pedestris. An analysis of metabolites revealed differences between the treatments, and while several metabolites markedly increased with cold acclimation, their concentrations were too low to have a significant effect on cold tolerance.

A minimalistic and optimized conveyor belt for neutral atoms.

Science.gov (United States)

Roy, Ritayan; Condylis, Paul C; Prakash, Vindhiya; Sahagun, Daniel; Hessmo, Björn

2017-10-20

Here we report of a design and the performance of an optimized micro-fabricated conveyor belt for precise and adiabatic transportation of cold atoms. A theoretical model is presented to determine optimal currents in conductors used for the transportation. We experimentally demonstrate a fast adiabatic transportation of Rubidium ( 87 Rb) cold atoms with minimal loss and heating with as few as three conveyor belt conductors. This novel design of a multilayered conveyor belt structure is fabricated in aluminium nitride (AlN) because of its outstanding thermal and electrical properties. This demonstration would pave a way for a compact and portable quantum device required for quantum information processing and sensors, where precise positioning of cold atoms is desirable.

Selective-field-ionization dynamics of a lithium m=2 Rydberg state: Landau-Zener model versus quantal approach

International Nuclear Information System (INIS)

Foerre, M.; Hansen, J.P.

2003-01-01

The selective-field-ionization (SFI) dynamics of a Rydberg state of lithium with magnetic quantum number m=2 is studied in detail based on two different theoretical models: (1) a close coupling integration of the Schroedinger equation and (2) the multichannel (incoherent) Landau-Zener (MLZ) model. The m=2 states are particularly interesting, since they define a border zone between fully adiabatic (m=0,1) and fully diabatic (m>2) ionization dynamics. Both sets of calculations are performed up to, and above, the classical ionization limit. It is found that the MLZ model is excellent in the description of the fully diabatic dynamics while certain discrepancies between the time dependent quantal amplitudes appear when the dynamics become involved. Thus, in this region, the analysis of experimental SFI spectra should be performed with care

Cold formability of steels

International Nuclear Information System (INIS)

Lafond, G.; Leclerq, G.; Moliexe, F.; Namdar, R.; Roesch, L.; Sanz, G.

1977-01-01

This work was essentially aimed to the study of the following three questions. Is it possible to assess the cold formability of steels using simple material properties as criteria. What values of mechanical properties can one expect to reach in cold formed parts. Are there simple ways of characterizing the speroidization treatments carried out on steels before cold forming operations. The present report describes the results obtained during this investigation. It is logically divided into three separate parts. Experimental study of cold formability in wire drawing. Influence of metallurgical variables on mechanical properties of high carbon cold drawn wires. Contribution to the study of characterization methods of cold forming steels subjected to a spheroidization heat treatment

Human whole body cold adaptation.

Science.gov (United States)

Daanen, Hein A M; Van Marken Lichtenbelt, Wouter D

2016-01-01

Reviews on whole body human cold adaptation generally do not distinguish between population studies and dedicated acclimation studies, leading to confusing results. Population studies show that indigenous black Africans have reduced shivering thermogenesis in the cold and poor cold induced vasodilation in fingers and toes compared to Caucasians and Inuit. About 40,000 y after humans left Africa, natives in cold terrestrial areas seems to have developed not only behavioral adaptations, but also physiological adaptations to cold. Dedicated studies show that repeated whole body exposure of individual volunteers, mainly Caucasians, to severe cold results in reduced cold sensation but no major physiological changes. Repeated cold water immersion seems to slightly reduce metabolic heat production, while repeated exposure to milder cold conditions shows some increase in metabolic heat production, in particular non-shivering thermogenesis. In conclusion, human cold adaptation in the form of increased metabolism and insulation seems to have occurred during recent evolution in populations, but cannot be developed during a lifetime in cold conditions as encountered in temperate and arctic regions. Therefore, we mainly depend on our behavioral skills to live in and survive the cold.

Searching for an Oscillating Massive Scalar Field as a Dark Matter Candidate Using Atomic Hyperfine Frequency Comparisons.

Science.gov (United States)

Hees, A; Guéna, J; Abgrall, M; Bize, S; Wolf, P

2016-08-05

We use 6 yrs of accurate hyperfine frequency comparison data of the dual rubidium and caesium cold atom fountain FO2 at LNE-SYRTE to search for a massive scalar dark matter candidate. Such a scalar field can induce harmonic variations of the fine structure constant, of the mass of fermions, and of the quantum chromodynamic mass scale, which will directly impact the rubidium/caesium hyperfine transition frequency ratio. We find no signal consistent with a scalar dark matter candidate but provide improved constraints on the coupling of the putative scalar field to standard matter. Our limits are complementary to previous results that were only sensitive to the fine structure constant and improve them by more than an order of magnitude when only a coupling to electromagnetism is assumed.

The impact of cold spells on mortality and effect modification by cold spell characteristics

Science.gov (United States)

Wang, Lijun; Liu, Tao; Hu, Mengjue; Zeng, Weilin; Zhang, Yonghui; Rutherford, Shannon; Lin, Hualiang; Xiao, Jianpeng; Yin, Peng; Liu, Jiangmei; Chu, Cordia; Tong, Shilu; Ma, Wenjun; Zhou, Maigeng

2016-12-01

In China, the health impact of cold weather has received little attention, which limits our understanding of the health impacts of climate change. We collected daily mortality and meteorological data in 66 communities across China from 2006 to 2011. Within each community, we estimated the effect of cold spell exposure on mortality using a Distributed Lag Nonlinear Model (DLNM). We also examined the modification effect of cold spell characteristics (intensity, duration, and timing) and individual-specific factors (causes of death, age, gender and education). Meta-analysis method was finally used to estimate the overall effects. The overall cumulative excess risk (CER) of non-accidental mortality during cold spell days was 28.2% (95% CI: 21.4%, 35.3%) compared with non-cold spell days. There was a significant increase in mortality when the cold spell duration and intensity increased or occurred earlier in the season. Cold spell effects and effect modification by cold spell characteristics were more pronounced in south China. The elderly, people with low education level and those with respiratory diseases were generally more vulnerable to cold spells. Cold spells statistically significantly increase mortality risk in China, with greater effects in southern China. This effect is modified by cold spell characteristics and individual-level factors.

Autoionization structure of nitric oxide (NO) at the first ionization limit

International Nuclear Information System (INIS)

Miescher, E.; Lee, Y.T.; California Univ., Berkeley; Guertler, P.

1977-12-01

A new and more detailed interpretation is given to the fine structure in the photoionization curve of cold NO observed by Ng, Mahan and Lee (J. Chem. Phys. 65 (1976) 1975). Resonances are assigned to autoionizing np and nd delta Rydberg levels which give prominent diffuse absorption bands in a spectrum recorded with the synchrotron radiation continuum. Δv [de

Theory and computation of the matrix elements of the full interaction of the electromagnetic field with an atomic state: Application to the Rydberg and the continuous spectrum

International Nuclear Information System (INIS)

Komninos, Yannis; Mercouris, Theodoros; Nicolaides, Cleanthes A.

2002-01-01

We develop practical formulas for the calculation of the matrix elements of the interaction of the electromagnetic field with an atomic state, beyond the long-wavelength approximation. The atom-plus-field Hamiltonian is chosen to have the multipolar form, containing the electric, paramagnetic, and diamagnetic operators. The final workable expressions include the interactions to all orders and are derived by first expanding the fields in partial waves. The electric-field operator reaches a constant value as the radial variable becomes large, contrary to the result of the electric-dipole approximation (EDA) where the value of the corresponding operator increases indefinitely. Applications are given for Rydberg states of hydrogen up to n=50 and for free-free transitions in a Coulomb potential. Such matrix elements are relevant to a number of real and virtual processes occurring during laser-atom interactions. The computation is done numerically, using a combination of analytic with numerical techniques. By comparing the results of the EDA with those of the exact treatment, it is shown that the former is inadequate in such cases. This finding has repercussions on the theory and understanding of the physics of quantum systems in high-lying Rydberg levels and wave packets or in scattering states

Cold/menthol TRPM8 receptors initiate the cold-shock response and protect germ cells from cold-shock-induced oxidation.

Science.gov (United States)

Borowiec, Anne-Sophie; Sion, Benoit; Chalmel, Frédéric; D Rolland, Antoine; Lemonnier, Loïc; De Clerck, Tatiana; Bokhobza, Alexandre; Derouiche, Sandra; Dewailly, Etienne; Slomianny, Christian; Mauduit, Claire; Benahmed, Mohamed; Roudbaraki, Morad; Jégou, Bernard; Prevarskaya, Natalia; Bidaux, Gabriel

2016-09-01

Testes of most male mammals present the particularity of being externalized from the body and are consequently slightly cooler than core body temperature (4-8°C below). Although, hypothermia of the testis is known to increase germ cells apoptosis, little is known about the underlying molecular mechanisms, including cold sensors, transduction pathways, and apoptosis triggers. In this study, using a functional knockout mouse model of the cold and menthol receptors, dubbed transient receptor potential melastatine 8 (TRPM8) channels, we found that TRPM8 initiated the cold-shock response by differentially modulating cold- and heat-shock proteins. Besides, apoptosis of germ cells increased in proportion to the cooling level in control mice but was independent of temperature in knockout mice. We also observed that the rate of germ cell death correlated positively with the reactive oxygen species level and negatively with the expression of the detoxifying enzymes. This result suggests that the TRPM8 sensor is a key determinant of germ cell fate under hypothermic stimulation.-Borowiec, A.-S., Sion, B., Chalmel, F., Rolland, A. D., Lemonnier, L., De Clerck, T., Bokhobza, A., Derouiche, S., Dewailly, E., Slomianny, C., Mauduit, C., Benahmed, M., Roudbaraki, M., Jégou, B., Prevarskaya, N., Bidaux, G. Cold/menthol TRPM8 receptors initiate the cold-shock response and protect germ cells from cold-shock-induced oxidation. © The Author(s).

Cold stress alters transcription in meiotic anthers of cold tolerant chickpea (Cicer arietinum L.).

Science.gov (United States)

Sharma, Kamal Dev; Nayyar, Harsh

2014-10-11

Cold stress at reproductive phase in susceptible chickpea (Cicer arietinum L.) leads to pollen sterility induced flower abortion. The tolerant genotypes, on the other hand, produce viable pollen and set seed under cold stress. Genomic information on pollen development in cold-tolerant chickpea under cold stress is currently unavailable. DDRT-PCR analysis was carried out to identify anther genes involved in cold tolerance in chickpea genotype ICC16349 (cold-tolerant). A total of 9205 EST bands were analyzed. Cold stress altered expression of 127 ESTs (90 up-regulated, 37 down-regulated) in anthers, more than two third (92) of which were novel with unknown protein identity and function. Remaining about one third (35) belonged to several functional categories such as pollen development, signal transduction, ion transport, transcription, carbohydrate metabolism, translation, energy and cell division. The categories with more number of transcripts were carbohydrate/triacylglycerol metabolism, signal transduction, pollen development and transport. All but two transcripts in these categories were up-regulated under cold stress. To identify time of regulation after stress and organ specificity, expression levels of 25 differentially regulated transcripts were also studied in anthers at six time points and in four organs (anthers, gynoecium, leaves and roots) at four time points. Limited number of genes were involved in regulating cold tolerance in chickpea anthers. Moreover, the cold tolerance was manifested by up-regulation of majority of the differentially expressed transcripts. The anthers appeared to employ dual cold tolerance mechanism based on their protection from cold by enhancing triacylglycerol and carbohydrate metabolism; and maintenance of normal pollen development by regulating pollen development genes. Functional characterization of about two third of the novel genes is needed to have precise understanding of the cold tolerance mechanisms in chickpea anthers.

Cough & Cold Medicine Abuse

Science.gov (United States)

... Videos for Educators Search English Español Cough & Cold Medicine Abuse KidsHealth / For Teens / Cough & Cold Medicine Abuse ... resfriado Why Do People Use Cough and Cold Medicines to Get High? There's an ingredient in many ...

Sub-nanometer distances and cluster shapes in dense hydrogen and in higher levels of hydrogen Rydberg matter by phase-delay spectroscopy

International Nuclear Information System (INIS)

Holmlid, Leif

2011-01-01

The inter-atomic distances in potassium clusters of Rydberg matter (RM) at excitation levels n B = 4–8 were recently measured by phase-delay spectroscopy (Holmlid, J Nanopart Res 12: 273, 2010). Excitation levels n B B = 1, 2, and 3 is found. Close-packing is the main structure both in planar and 3D clusters. Planar clusters are only observed for n B = 1 and 3, while 3D clusters are found in excitation levels n B = 1, 2 and 3. The cluster–cluster distance in stacks of planar clusters for n B = 2 and 3 is now observed for the first time.

Jagiellonian University Advances in Ps Manipulations and Laser Studies in the AEgIS Experiment

CERN Document Server

Caravita, R; Amsler, C; Bonomi, G; Brusa, R S; Caccia, M; Castelli, F; Cerchiari, G; Comparat, D; Consolati, G; Demetrio, A; Di Noto, L; Doser, M; Evans, C; Ferragut, R; Fesel, J; Fontana, A; Gerber, S; Giammarchi, M; Gligorova, A; Guatieri, F; Haider, S; Hinterberger, A; Holmestad, H; Kellerbauer, A; Khalidova, O; Krasnický, D; Lagomarsino, V; Lansonneur, P; Lebrun, P; Malbrunot, C; Mariazzi, S; Marton, J; Matveev, V; Mazzotta, Z; Müller, S R; Nebbia, G; Nedelec, P; Oberthaler, M; Pacifico, N; Pagano, D; Penasa, L; Petracek, V; Prelz, F; Prevedelli, M; Ravelli, L; Rienäcker, B; Robert, J; Røhne, O M; Rotondi, A; Sandaker, H; Santoro, R; Smestad, L; Sorrentino, F; Testera, G; Tietje, I; Widmann, E; Yzombard, P; Zimmer, C; Zmeskal, J; Zurlo, N

2017-01-01

Positronium (Ps), the unstable bound state of electron and positron, is a valuable system for neutral antimatter spectroscopic studies and for antihydrogen production. Forming a pulsed beam cold antihydrogen using charge-exchange with the Rydberg Ps is the goal of the AEgIS Collaboration, which aims to measure gravity on neutral antimatter. Recent results achieved in producing, manipulating and studying Ps are summarized. Ps has been first produced with mesoporous silica targets in a reflection geometry. Spectroscopy of Ps n = 3 state has been conducted, yielding as a byproduct an independent estimate of the produced Ps temperature. Efficient laser excitation to the Rydberg levels was then achieved, validating the proof-of-concept of AEgIS. Subsequently, production of Ps from a new class of transmission targets was also achieved, opening the possibility for future experiments.

Control of Goos-Hänchen shift via input probe field intensity

Science.gov (United States)

Ziauddin; Lee, Ray-Kuang; Qamar, Sajid

2016-11-01

We suggest a scheme to control Goos-Hänchen (GH) shift in an ensemble of strongly interacting Rydberg atoms, which act as super-atoms due to the dipole blockade mechanism. The ensemble of three-level cold Rydberg-dressed (87Rb) atoms follows a cascade configurations where two fields, i.e, a strong control and a weak field are employed [D. Petrosyan, J. Otterbach, and M. Fleischhauer, Phys. Rev. Lett. 107, 213601 (2011)]. The propagation of probe field is influenced by two-photon correlation within the blockade distance, which are damped due to the saturation of super-atoms. The amplitude of GH shift in the reflected light depends on the intensity of probe field. We observe large negative GH shift in the reflected light for small values of the probe field intensities.

Commemoration of a cold war

DEFF Research Database (Denmark)

Farbøl, Rosanna

2015-01-01

This article brings together the fields of Cold War studies and memory studies. In Denmark, a remarkable institutionalisation of Cold War memory has taken place in the midst of a heated ideological battle over the past and whether to remember the Cold War as a ‘war’. Using Danish Cold War museums...... and heritage sites as case studies, this article sheds new light on the politics of history involved in Cold War commemoration. It suggests that the Cold War is commemorated as a war, yet this war memory is of a particular kind: it is a war memory without victims....