WorldWideScience

Sample records for charge state ion

  1. High-charge-state ion sources

    International Nuclear Information System (INIS)

    Sources of high charge state positive ions have uses in a variety of research fields. For heavy ion particle accelerators higher charge state particles give greater acceleration per gap and greater bending strength in a magnet. Thus higher energies can be obtained from circular accelerators of a given size, and linear accelerators can be designed with higher energy gain per length using higher charge state ions. In atomic physics the many atomic transitions in highly charged ions supplies a wealth of spectroscopy data. High charge state ion beams are also used for charge exchange and crossed beam experiments. High charge state ion sources are reviewed

  2. Charge transfer processes of low charge state heavy ions

    International Nuclear Information System (INIS)

    In this paper, some aspects of the collision processes of accelerated heavy ions in very low charge state is reviewed, and the beam loss due to such collisions is estimated. The processes included in ion-atom collisions are electron capture, the electron stripping of ions, and target ionization. The stripping cross sections decrease slowly at high energy, and are much larger than the electron capture cross sections. At low energy, the electron capture is dominant, and this process plays a principal role near ion sources and preacceleration regions. This has not been taken into account properly. In order to keep the beam loss less than 0.1 percent, it is estimated that the average vacuum of about 10-7 to 10-8 Torr is required. An empirical formula to calculate the stripping cross sections of heavy ions in low charge state in collisions is derived. The beam loss due to ion-atom collisions can be estimated. The charge transfer and stripping processes in ion-ion collisions are also discussed. The typical processes in ion-ion collisions are almost same as those in ion-atom collisions. In order to minimize the ion beam loss due to charge-changing processes, it is important to choose the heavy ions with closed shell configurations, which correspond to the slightly more ionized states than the singly ionized state. (Kato, T.)

  3. Charge states of ions, and mechanisms of charge ordering transitions

    International Nuclear Information System (INIS)

    To gain insight into the mechanism of charge ordering transitions, which conventionally are pictured as a disproportionation of an ion M as 2Mn+→M(n+1)+ + M(n−1)+, we (1) review and reconsider the charge state (or oxidation number) picture itself, (2) introduce new results for the putative charge ordering compound AgNiO2 and the dual charge state insulator AgO, and (3) analyze the cationic occupations of the actual (not formal) charge, and work to reconcile the conundrums that arise. We establish that several of the clearest cases of charge ordering transitions involve no disproportion (no charge transfer between the cations, and hence no charge ordering), and that the experimental data used to support charge ordering can be accounted for within density functional-based calculations that contain no charge transfer between cations. We propose that the charge state picture retains meaning and importance, at least in many cases, if one focuses on Wannier functions rather than atomic orbitals. The challenge of modeling charge ordering transitions with model Hamiltonians isdiscussed. (paper)

  4. Charge-state evolution of highly charged ions transmitted through microcapillaries

    OpenAIRE

    Tokesi, K.; Wirtz, Ludger; Lemell, C.; Burgdorfer, J.

    2000-01-01

    The charge-state evolution of highly charged ions transmitted through microcapillaries is studied theoretically by a classical trajectory Monte Carlo simulation.: The interaction of highly charged ions with the internal surface of the capillary is treated within the framework of dielectric response theory. We analyze the distance of closest approach and the angular distributions of the highly charged ions at the exit of the microcapillary. We find the charge-state fraction of transmitted N6+ ...

  5. Charge-State Distributions of Accelerated ^{48}Ca Ions

    CERN Document Server

    Skobelev, N K; Astabatyan, R A; Vincour, J; Kulko, A A; Lobastov, S P; Lukyanov, S M; Markaryan, E R; Maslov, V A; Penionzhkevich, Yu E; Sobolev, Yu G; Ugryumov, V Yu

    2003-01-01

    A stepped pole broad-range magnetic analyzer has been used to measure the charge-state distributions of accelerated ^{48}Ca ions at the two incident energies 242.8 and 264.5 MeV after passing through thin carbon or gold target foils. The measured charge-state distributions and the mean equilibrium charge of the ^{48}Ca ions are compared with various calculations. It has been shown that the calculations can be used only for evaluation purposes.

  6. Equilibrium charge state distributions of high energy heavy ions

    International Nuclear Information System (INIS)

    Equilibrium charge state fractions have been measured for N, O, Ne, S, Ar and Kr ions at 1.04 MeV/nucleon after passing through various stripping materials. Further data were obtained at higher energy for S ions (4.12 MeV/nucleon) and Ar ions (4.12 and 9.6 MeV/nucleon). The mean charge fractions can be fitted to universal curves for both solid and gaseous strippers. Measurements of the equilibrium fraction of krypton ions at 1.04 MeV/nucleon passing through heavy vapours have shown that a higher average charge state is obtained than for lighter gaseous strippers. (Auth.)

  7. A high charge state heavy ion beam source for HIF

    International Nuclear Information System (INIS)

    A high current low emittance high charge state heavy ion beam source is being developed. This is designed to deliver HIF (heavy ion fusion) driver accelerator scale beam. Using high-charge-state beam in a driver accelerator for HIF may increase the acceleration efficiency, leading to a reduction in the driver accelerator size and cost. The proposed source system which consists of the gas beam electron stripper followed by a high charge state beam separator, can be added to existing single charge state, low emittance, high brightness ion sources and injectors. We shall report on the source physics design using 2D beam envelope simulations and experimental feasibility studies' results using a neutral gas stripper and a beam separator at the exit of the LBL 2 MV injector

  8. Formation of High Charge State Heavy Ion Beams with intense Space Charge

    International Nuclear Information System (INIS)

    High charge-state heavy-ion beams are of interest and used for a number of accelerator applications. Some accelerators produce the beams downstream of the ion source by stripping bound electrons from the ions as they pass through a foil or gas. Heavy-ion inertial fusion (HIF) would benefit from low-emittance, high current ion beams with charge state >1. For these accelerators, the desired dimensionless perveance upon extraction from the emitter is ∼10-3, and the electrical current of the beam pulse is ∼1 A. For accelerator applications where high charge state and very high current are desired, space charge effects present unique challenges. For example, in a stripper, the separation of charge states creates significant nonlinear space-charge forces that impact the beam brightness. We will report on the particle-in-cell simulation of the formation of such beams for HIF, using a thin stripper at low energy.

  9. Multiple charge states of titanium ions in laser produced plasma

    International Nuclear Information System (INIS)

    An intense laser radiation (1012 to 1014 W/cm-2) focused on the solid target creates a hot (≥ 1 KeV) and dense plasma having high ionization state. The multiple charged ions with high current densities produced during laser matter interaction have potential application in accelerators as an ion source. This paper presents generation and detection of highly stripped titanium ions (Ti) in laser produced plasma. An Nd:glass laser (KAMETRON) delivering 50 J energy (λ = 0.53 μm) in 2.5 ns was focused onto a titanium target to produce plasma. This plasma was allowed to drift across a space ∼ 3m through a diagnostic hole in the focusing mirror before ions are finally detected with the help of electrostatic ion analyzer. Maximum current density was detected for the charge states of +16 and +17 of Ti ions for laser intensity of ∼ 1014 W/cm-2. (author)

  10. Ion temperature effects on ion charge-state distributions of an electron cyclotron resonant ion source

    International Nuclear Information System (INIS)

    A method is described for determining ion cyclotron resonance (ICR) heating effects on multiply charged-ion energy distributions using a Monte Carlo fit to experimental time-of-flight spectrometer data. The method is general but is used here specifically to separate the effects of plasma ambipolar potential spread and ion temperature in an electron cyclotron resonance (ECR) heated magnetic mirror ion source (MIMI) [Phys. Fluids 28, 3116 (1985)]. A steady-state equilibrium model is also developed that models the relevant atomic processes occurring in MIMI plasmas. This model and the Monte Carlo analysis are used to relate the effect of midplane ICR heating on end loss ion charge state distributions to its effect on the confined ion distributions. The model allows for collisional, moderately collisional, and collisionless confinement, specific to each charge state in the distribution. Both experiment and modeling show that increased ion temperature causes a shift to lower-Z ion populations in both the confined and end loss charge-state distributions

  11. The charge state of the ions produced by a saddle field ion source

    International Nuclear Information System (INIS)

    The thesis is concerned with an analysis of the charge state and energy of the ions produced by a saddle field ion source, and its application to the measurement of the sputtering yield. The subject is discussed under the topic headings: production of multicharged ions, saddle field ion sources, experimental conditions, ionic charge state, energy for argon, and sputtering yield of gold for Ar+ and Ar2+ ions. (U.K.)

  12. Charge-state-specific EUV spectra of Xe ions

    International Nuclear Information System (INIS)

    Charge state specific extreme ultraviolet spectra from xenon ions have been recorded at Tokyo Metropolitan University. The Electron Cyclotron Resonance Source spectra were produced from charge exchange collisions between the xenon ions and rare gas target atoms. Atomic structure calculations were performed for Xe 16+ − Xe20+ using the Hartree-Fock with Configuration Interaction code of Cowan and showed that the spectra arise from 4p-4d and 4d-4f transitions. In addition it was necessary to allow for selective capture processes that occur in these slow collisions. The energies of the capture states involved in the single electron process are estimated using the classical over barrier model.

  13. Synchrotron injectors based on high charge state ion sources

    International Nuclear Information System (INIS)

    The performance of any injector contemplated to replace the electrostatic tandem accelerators some time in the future should evidently match or surpass the characteristics of the tandems. It is a fortunate coincidence that the performance of the BNL tandem satisfies in most respects the requirements of the proposed collider, although originally tandems were not built with this application in mind. Requests for heavy ion beams with parameters suitable for injection into the rings of a heavy ion collider have appeared rather recently, at a stage when the high charge state ion sources, which in principle are capable of producing many ion species, have not yet reached such a level of performance. Therefore, consideration of such sources as part of a future injector replacing the tandem accelerators will have to rely on the extrapolation of results from existing models, developed for a different purpose. At the same time, present and future collider requirements for heavy ion beams should serve as a stimulus for the development of sources producing ions with adequate charge states and intensities. Injectors based on such sources may present a better alternative than the tandem accelerators because a higher charge-to-mass ratio of ions from the source results in a more efficient and less costly accelerator. In this report, two candidates for a high charge state, heavy ion source will be considered: an EBIS and an ECR. Other approaches, e.g. laser ion sources, are much further away in the development of a device to be used in a synchrotron injector. 25 refs., 7 figs., 4 tabs

  14. High Intensity High Charge State ECR Ion Sources

    CERN Document Server

    Leitner, Daniela

    2005-01-01

    The next-generation heavy ion beam accelerators such as the proposed Rare Isotope Accelerator (RIA), the Radioactive Ion Beam Factory at RIKEN, the GSI upgrade project, the LHC-upgrade, and IMP in Lanzhou require a great variety of high charge state ion beams with a magnitude higher beam intensity than currently achievable. High performance Electron Cyclotron Resonance (ECR) ion sources can provide the flexibility since they can routinely produce beams from hydrogen to uranium. Over the last three decades, ECR ion sources have continued improving the available ion beam intensities by increasing the magnetic fields and ECR heating frequencies to enhance the confinement and the plasma density. With advances in superconducting magnet technology, a new generation of high field superconducting sources is now emerging, designed to meet the requirements of these next generation accelerator projects. The talk will briefly review the field of high performance ECR ion sources and the latest developments for high intens...

  15. Vacuum improvements for ultra high charge state ion acceleration

    International Nuclear Information System (INIS)

    The installation of a second cryo panel has significantly improved the vacuum in the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. The neutral pressure in the extraction region decreased from 1.2 x 10-6 down to about 7 x 10-7 Torr. The vacuum improvement reduces beam loss from charge changing collisions and enhances the cyclotron beam transmission, especially for the high charge state heavy ions. Tests with improved vacuum show the cyclotron transmission increased more than 50% (from 5.7% to 9.0%) for a Xe27+ at 603 MeV, more than doubled for a Bi41+ beam (from 1.9% to 4.6%) at 904 MeV and tripled for a U47+ beam (from 1.2% to 3.6%) at 1,115 MeV. At about 5 NeV/nucleon 92 enA (2.2 pnA) for Bi41+ and 14 enA (0.3 pnA) for U47+ were extracted ut of the 88-Inch Cyclotron Ion beams with charge states as high as U64+ have been produced by the LBNL AECR-U ion source and accelerated through the cyclotron for the first time. The beam losses for a variety of ultra high charge state ions were measured as a function of cyclotron pressure and compared with the calculations from the existing models

  16. High-Intensity, High Charge-State Heavy Ion Sources

    CERN Document Server

    Alessi, J

    2004-01-01

    There are many accelerator applications for high intensity heavy ion sources, with recent needs including dc beams for RIA, and pulsed beams for injection into synchrotrons such as RHIC and LHC. The present status of sources producing high currents of high charge state heavy ions will be reviewed. These sources include ECR, EBIS, and Laser ion sources. The benefits and limitations for these type sources will be described, for both dc and pulsed applications. Possible future improvements in these type sources will also be discussed.

  17. A vacuum spark ion source: High charge state metal ion beams

    Energy Technology Data Exchange (ETDEWEB)

    Yushkov, G. Yu., E-mail: gyushkov@mail.ru; Nikolaev, A. G.; Frolova, V. P. [High Current Electronics Institute, Siberian Branch of the Russian Academy of Science, Tomsk 634055 (Russian Federation); Oks, E. M. [High Current Electronics Institute, Siberian Branch of the Russian Academy of Science, Tomsk 634055 (Russian Federation); Tomsk State University of Control System and Radioelectronics, Tomsk 634050 (Russian Federation)

    2016-02-15

    High ion charge state is often important in ion beam physics, among other reasons for the very practical purpose that it leads to proportionately higher ion beam energy for fixed accelerating voltage. The ion charge state of metal ion beams can be increased by replacing a vacuum arc ion source by a vacuum spark ion source. Since the voltage between anode and cathode remains high in a spark discharge compared to the vacuum arc, higher metal ion charge states are generated which can then be extracted as an ion beam. The use of a spark of pulse duration less than 10 μs and with current up to 10 kA allows the production of ion beams with current of several amperes at a pulse repetition rate of up to 5 pps. We have demonstrated the formation of high charge state heavy ions (bismuth) of up to 15 + and a mean ion charge state of more than 10 +. The physics and techniques of our vacuum spark ion source are described.

  18. A vacuum spark ion source: High charge state metal ion beams

    International Nuclear Information System (INIS)

    High ion charge state is often important in ion beam physics, among other reasons for the very practical purpose that it leads to proportionately higher ion beam energy for fixed accelerating voltage. The ion charge state of metal ion beams can be increased by replacing a vacuum arc ion source by a vacuum spark ion source. Since the voltage between anode and cathode remains high in a spark discharge compared to the vacuum arc, higher metal ion charge states are generated which can then be extracted as an ion beam. The use of a spark of pulse duration less than 10 μs and with current up to 10 kA allows the production of ion beams with current of several amperes at a pulse repetition rate of up to 5 pps. We have demonstrated the formation of high charge state heavy ions (bismuth) of up to 15 + and a mean ion charge state of more than 10 +. The physics and techniques of our vacuum spark ion source are described

  19. A vacuum spark ion source: High charge state metal ion beams

    Science.gov (United States)

    Yushkov, G. Yu.; Nikolaev, A. G.; Oks, E. M.; Frolova, V. P.

    2016-02-01

    High ion charge state is often important in ion beam physics, among other reasons for the very practical purpose that it leads to proportionately higher ion beam energy for fixed accelerating voltage. The ion charge state of metal ion beams can be increased by replacing a vacuum arc ion source by a vacuum spark ion source. Since the voltage between anode and cathode remains high in a spark discharge compared to the vacuum arc, higher metal ion charge states are generated which can then be extracted as an ion beam. The use of a spark of pulse duration less than 10 μs and with current up to 10 kA allows the production of ion beams with current of several amperes at a pulse repetition rate of up to 5 pps. We have demonstrated the formation of high charge state heavy ions (bismuth) of up to 15 + and a mean ion charge state of more than 10 +. The physics and techniques of our vacuum spark ion source are described.

  20. MULTIPLY CHARGED IONS COLLISIONS WITH ATOMS INTO EXCITED STATES

    Institute of Scientific and Technical Information of China (English)

    PanGuangyan

    1990-01-01

    The emission spectra in collisions between Ions and Atoms have been measured by an Optical Multichannel Analysis System (OMA).The experimental results demonstrate that there are two channels of excitation in collision between single charged ions and atoms and three channels of excitation in collision between double charged ions and atoms.Emission cross cestions and excitation cross sections have been obtained.K.Kadota et al and R.Shingal et al suggested that,under the appropriate conditions,the H42+-Li and He2++Na collision systems can be used efficiently to produce a laser of Lyman-α(30,4nm) and Lyman-β(25.6nm)lines via cascade to He+(2P)state.

  1. Effects of Solvent on the Maximum Charge State and Charge State Distribution of Protein Ions Produced by Electrospray Ionization

    OpenAIRE

    Iavarone, Anthony T.; Jurchen, John C.; Williams, Evan R.

    2000-01-01

    The effects of solvent composition on both the maximum charge states and charge state distributions of analyte ions formed by electrospray ionization were investigated using a quadrupole mass spectrometer. The charge state distributions of cytochrome c and myoglobin, formed from 47%/50%/3% water/solvent/acetic acid solutions, shift to lower charge (higher m/z) when the 50% solvent fraction is changed from water to methanol, to acetonitrile, to isopropanol. This is also the order of increasing...

  2. Charge state distribution analysis of Al and Pb ions from the laser ion source at IMP

    International Nuclear Information System (INIS)

    A prototype laser ion source that could demonstrate the possibility of producing intense pulsed high charge state ion beams has been established with a commercial Nd:YAG laser (Emax=3 J, 1064 nm, 8-10 ns) to produce laser plasma for the research of Laser Ion Source (LIS). At the laser ion source test bench, high purity (99.998%) aluminum and lead targets have been tested for laser plasma experiment. An Electrostatic Ion Analyzer (EIA) and Electron Multiply Tube (EMT) detector were used to analyze the charge state and energy distribution of the ions produced by the laser ion source. The maximum charge states of Al12+ and Pb7+ were achieved. The results will be presented and discussed in this paper. (authors)

  3. Charge state distribution analysis of Al and Pb ions from the laser ion source at IMP

    CERN Document Server

    Shan, Sha; Zhang-Min, Li; Xiao-Hong, Guo; Lun-Cai, Zhou; Guo-Zhu, Cai; Liang-ting, Sun; Xue-Zhen, Zhang; Huan-Yu, Zhao; Xi-Meng, Chen; Hong-Wei, Zhao

    2013-01-01

    A prototype laser ion source that could demonstrate the possibility of producing intense pulsed high charge state ion beams has been established with a commercial Nd:YAG laser (E max = 3 J, 1064 nm, 8-10 ns) to produce laser plasma for the research of Laser Ion Source (LIS). At the laser ion source test bench, high purity (99.998 %) aluminum and lead targets have been tested for laser plasma experiment. An Electrostatic Ion Analyzer (EIA) and Electron Multiply Tube (EMT) detector were used to analyze the charge state and energy distribution of the ions produced by the laser ion source. The maximum charge states of Al12+ and Pb7+ were achieved. The results will be presented and discussed in this paper.

  4. Analysis of Ion Charge States in Solar Wind and CMEs

    Indian Academy of Sciences (India)

    Arati Dasgupta; J. M. Laming

    2008-03-01

    We discuss needs in dielectronic recombination data motivated by recent work directed at a quantitative understanding of ion charge states of various elements observed in situ in the solar wind and CMEs. The competing processes of ionization and recombination lead to departures from collision ionization equilibrium. The use of this as a diagnostic of acceleration and heating processes of the solar wind and CMEs is sensitive to the accuracy of the atomic rates in a way that steady state ionization equilibrium plasmas are not. The most pressing need is dielectronic recombination rates for ions Fe8+-12+. These are among the dominant species observed in various regions of the solar wind and CMEs, and in remotely sensed EUV spectra.

  5. Low charge state heavy ion production with sub-nanosecond laser

    International Nuclear Information System (INIS)

    We have investigated laser ablation plasma of various species using nanosecond and sub-nanosecond lasers for both high and low charge state ion productions. We found that with sub-nanosecond laser, the generated plasma has a long tail which has low charge state ions determined by an electrostatic ion analyzer even under the laser irradiation condition for highly charged ion production. This can be caused by insufficient laser absorption in plasma plume. This property might be suitable for low charge state ion production. We used a nanosecond laser and a sub-nanosecond laser for low charge state ion production to investigate the difference of generated plasma using the Zirconium target

  6. Low charge state heavy ion production with sub-nanosecond laser

    Energy Technology Data Exchange (ETDEWEB)

    Kanesue, T., E-mail: tkanesue@bnl.gov; Okamura, M. [Collider-Accelerator Department, Brookhaven National Laboratory, Upton, New York 11973 (United States); Kumaki, M. [Research Institute for Science and Engineering, Waseda University, Tokyo 169-8555 (Japan); Nishina Center for Accelerator-Based Science, RIKEN, Saitama 351-0198 (Japan); Ikeda, S. [Nishina Center for Accelerator-Based Science, RIKEN, Saitama 351-0198 (Japan); Interdisciplinary Graduate School of Science and Engineering, Tokyo Institute of Technology, Kanagawa 226-8503 (Japan)

    2016-02-15

    We have investigated laser ablation plasma of various species using nanosecond and sub-nanosecond lasers for both high and low charge state ion productions. We found that with sub-nanosecond laser, the generated plasma has a long tail which has low charge state ions determined by an electrostatic ion analyzer even under the laser irradiation condition for highly charged ion production. This can be caused by insufficient laser absorption in plasma plume. This property might be suitable for low charge state ion production. We used a nanosecond laser and a sub-nanosecond laser for low charge state ion production to investigate the difference of generated plasma using the Zirconium target.

  7. Low charge state heavy ion production with sub-nanosecond laser

    Science.gov (United States)

    Kanesue, T.; Kumaki, M.; Ikeda, S.; Okamura, M.

    2016-02-01

    We have investigated laser ablation plasma of various species using nanosecond and sub-nanosecond lasers for both high and low charge state ion productions. We found that with sub-nanosecond laser, the generated plasma has a long tail which has low charge state ions determined by an electrostatic ion analyzer even under the laser irradiation condition for highly charged ion production. This can be caused by insufficient laser absorption in plasma plume. This property might be suitable for low charge state ion production. We used a nanosecond laser and a sub-nanosecond laser for low charge state ion production to investigate the difference of generated plasma using the Zirconium target.

  8. High ion charge states in a high-current, short-pulse, vacuum ARC ion sources

    Energy Technology Data Exchange (ETDEWEB)

    Anders, A.; Brown, I.; MacGill, R.; Dickinson, M. [Lawrence Berkeley National Lab., CA (United States)

    1996-08-01

    Ions of the cathode material are formed at vacuum arc cathode spots and extracted by a grid system. The ion charge states (typically 1-4) depend on the cathode material and only little on the discharge current as long as the current is low. Here the authors report on experiments with short pulses (several {mu}s) and high currents (several kA); this regime of operation is thus approaching a more vacuum spark-like regime. Mean ion charge states of up to 6.2 for tungsten and 3.7 for titanium have been measured, with the corresponding maximum charge states of up to 8+ and 6+, respectively. The results are discussed in terms of Saha calculations and freezing of the charge state distribution.

  9. Charge-state-dependent energy loss of slow ions. I. Experimental results on the transmission of highly charged ions

    Science.gov (United States)

    Wilhelm, Richard A.; Gruber, Elisabeth; Smejkal, Valerie; Facsko, Stefan; Aumayr, Friedrich

    2016-05-01

    We report on energy loss measurements of slow (v ≪v0 ), highly charged (Q >10 ) ions upon transmission through a 1-nm-thick carbon nanomembrane. We emphasize here the scaling of the energy loss with the velocity and charge exchange or loss. We show that a weak linear velocity dependence exists, whereas charge exchange dominates the kinetic energy loss, especially in the case of a large charge capture. A universal scaling of the energy loss with the charge exchange and velocity is found and discussed in this paper. A model for charge-state-dependent energy loss for slow ions is presented in paper II in this series [R. A. Wilhelm and W. Möller, Phys. Rev. A 93, 052709 (2016), 10.1103/PhysRevA.93.052709].

  10. Calculation of ion charge-state distribution in ECR ion sources

    International Nuclear Information System (INIS)

    Starting with the pioneering efforts of Y. Yongen (Louvain-la-Neuve, Belgium) a code has been developed to calculate the equilibrium ion charge-state distribution for electron-cyclotron resonance source (ECR) ion sources. Production of ions is caused by the impact ionization of the charge gas from ECR-heated electrons of a few keV. Loss of an ion of a given charge state is from charge exchange and radiative recombination. Ultimately, the ion flows out of the minimum-B containment region. The ion confinement times are calculated using an ion-trap-potential model which is based upon modeling calculations done at Lawrence Livermore National Laboratory (LLNL) for the Tandem Mirror Machine. Using this model requires the self-consistent determination of the trap potential and thermal electron density in the plasma. Code inputs are gas natural density, hot-electron temperature and density, ion temperature, cold-electron temperature, mirror ratio, physical dimensions, and atomic-physics data. Other than that there are no adjustable parameters. Results of comparison of calculations with the limited available data are reasonable

  11. On the physics of high charge state ion production in ECR ion sources

    International Nuclear Information System (INIS)

    Full text: In a previous research we have demonstrated that metal-dielectric (MD) structures have high capabilities of to enhance the high-charge-state ion production in ECR Ion Sources. In order to explain this effect, dedicated experiments have been performed, in which changes of main plasma parameters in the presence of a MD structure have been observed and an explanation for the mechanism of 'MD-effect' was given. In this contribution we present a new experiment, where we have concentrated on the question whether the effect of the high-charge-state enhancement by the MD structures is due to the presence of just a dielectric layer in the plasma chamber (e.g. working simply as a breaking of the non ambipolar wall currents) or whether details of the structure of the MD-layer play an essential role. By comparing ion charge state distributions (CSD) and Bremsstrahlung spectra for two MD cylinders, of drastically different layer thicknesses, the importance of the MD effect, and hence of the detailed structure of this type of layer for the production of very highly charged ions is demonstrated. The effect of the two different MD cylinders on the charge state distributions (CSD) of extracted argon ion is presented. It is obvious that both cylinders influence the CSD in a totally different manner. Whereas the thin MD-liner serves to strongly enhance the currents of ions with charge states higher than 9+, the thick MD-liner acted in the opposite way, i.e. enhancing the lower charge states. The experiments reported here demonstrate the role of the MD physics for obtaining an enhanced high charge state ion production in ECRIS. Following established scaling laws, the observed shift of the mean charge state in this experiment is equivalent to a frequency upgrade of an ECRIS from e.g. 14 GHZ to 18 GHz. It has also been demonstrated that than the simple fact of restoring ambipolarity by breaking the Simon short circuits cannot explain this effect. Therefore, the method may

  12. Production of high charge state ions with the Advanced Electron Cyclotron Resonance Ion Source at LBNL

    International Nuclear Information System (INIS)

    Production of high charge state ions with the Advanced Electron Cyclotron Resonance ion source (AECR) at Lawrence Berkeley National Laboratory (LBNL) has been significantly improved by application of various new techniques. Heating the plasma simultaneously with microwaves of two frequencies (10 and 14 GHz) has increased the production of very high charge state heavy ions. The two-frequency technique provides extra electron cyclotron resonance heating zone as compared to the single-frequency heating and improves the heating of the plasma electrons. Aluminum oxide on the plasma chamber surface improves the production of cold electrons at the chamber surfaces and increases the performance of the AECR. Fully stripped argon ions, ≥5 enA, were produced and directly identified by the source charge state analyzing system. High charge state ion beams of bismuth and uranium, such as 209Bi51+ and 238U53+, were produced by the source and accelerated by the 88-in. cyclotron to energies above 6 MeV/nucleon for the first time. copyright 1996 American Institute of Physics

  13. Electron capture to autoionizing states of multiply charged ions

    International Nuclear Information System (INIS)

    The present thesis investigates electron capture reactions resulting from slow collisions (V q+) and neutral gas targets (B). The energy spectra of the emitted electrons are measured; detection angle is 500. Mainly, autoionizing double capture resulting from collisions with two-electron targets (He, H2) is studied; then, the emitted electrons stem from doubly excited projectile states. The projectiles used are bare C6+, the H-like and He-like ions of C, N and O, He-like Ne8+ and Ne-like Ar8+. Excited metastable projectiles used are C5+(2s), He-like projectiles Aq+(1s2s3S) and Ar8+(...2p53s). Comparison is made with the predictions of a recently proposed extended classical barrier model, that was developed in connection with the work. This model assumes sequential capture of the electrons ('two-step' process); it predicts the realized binding enegies of the captured electrons - which may be directly determined from the autoionization spectra using only the projectile charge, the ionization potentials of the target and the collision velocity as parameters. No adjustable parameter enters into the calculations. The term energies and decay modes of the highly excited product ions themselves are studied. Generally, the autoionizing decay of these states is found to proceed preferentially to the directly adjacent lower singly excited state. Experimental evidence is presented, that triply excited states decay by successive emission of two electrons, whenever this is energetically possible. Finally, the L-MM decay in few-electron systems is considered. 314 refs.; 96 figs.; 29 tabs

  14. Production of high charge state ions with the Advanced Electron Cyclotron Resonance ion source at LBNL

    International Nuclear Information System (INIS)

    Production of high charge state ions with the Advanced Electron Cyclotron Resonance ion source (AECR) at Lawrence Berkeley National Laboratory (LBNL) has been significantly improved by application of various new techniques. Heating the plasma simultaneously with microwaves of two frequencies (10 and 14 GHz) has increased the production of very high charge state heavy ions. The two-frequency technique provides extra electron cyclotron resonance heating zone as compared to the single-frequency heating and improves the heating of the plasma electrons. Aluminum oxide on the plasma chamber surface improves the production of cold electrons at the chamber surfaces and increases the performance of the AECR. Fully stripped argon ions, > 5 enA, were produced and directly identified by the source charge state analyzing system. High charge state ion beams of bismuth and uranium, such as 209Bi51+ and 238U53+, were produced by the source and accelerated by the 88-Inch Cyclotron to energies above 6 MeV/nucleon for the first time. To further increase the production of high charge state ions to support the nuclear science research programs at the 88-Inch Cyclotron, an upgrade is taking place to increase the AECR magnetic field strengths and mirror ratios to improve the plasma confinement. Conceptual design is underway for a 3rd Generation ECR that uses superconducting magnets to reach higher magnetic field strengths and higher mirror ratios, high secondary emission chamber walls to increase the yield of cold electrons at the chamber surfaces and microwaves of multiple frequencies to improve plasma heating

  15. Charge State Evolution of Uranium in Electron Beam Ion Trap

    Institute of Scientific and Technical Information of China (English)

    LIU Ya-Feng; YAO Ke; Roger Hutton; ZOU Ya-Ming

    2005-01-01

    @@ We present a calculation scheme with significant modifications and improvements for determining the ionization balance and the ion temperature evolution in an electron beam ion trap (EBIT). The scheme is applied to uranium and nitrogen ions using a specific set of EBIT operating parameters. The calculation results are compared to the experimental data. Rates for the individual atomic processes in EBIT, especially single and multiple charge exchange processes, are discussed. The time evolution of the ion temperatures for uranium and its coolant nitrogen are also given.

  16. High charge-state ion beam production from a laser ion source

    International Nuclear Information System (INIS)

    The high current, high charge-state ion beam which can be extracted from a laser produced plasma is well suited, after initial acceleration, for injection into synchrotrons. At CERN, the production of a heavy ion beam using such a source is studied. A 60 mA pulse of a mixture of high charge state tantalum or lead ions of 5 μs duration has been extracted at 59 kV. The resulting beam emittance and energy spread were measured. A Low Energy Beam Transport system (LEBT) consisting of two pulsed solenoids is used to match the beam to a four-rod Radio Frequency Quadrupole (RFQ). Preliminary results are given for the acceleration of the beam by an RFQ, designed for the acceleration of 10 mA of Ta16+ to an energy of 100 keV/u. (author)

  17. Heavy-Ion Beam Acceleration of Two-Charge States from an Ecr Ion Source

    OpenAIRE

    Ostroumov, P. N.; Shepard, K. W.; Aseev, V. N.; Kolomiets, A. A.

    2000-01-01

    This paper describes a design for the front end of a superconducting (SC) ion linac which can accept and simultaneously accelerate two charge states of uranium from an ECR ion source. This mode of operation increases the beam current available for the heaviest ions by a factor of two. We discuss the 12 MeV/u prestripper section of the Rare Isotope Accelerator (RIA) driver linac including the LEBT, RFQ, MEBT and SC sections, with a total voltage of 112 MV. The LEBT consists of two bunchers and...

  18. Temporal evolution of ion energy distribution functions and ion charge states of Cr and Cr-Al pulsed arc plasmas

    International Nuclear Information System (INIS)

    To study the temporal evolution of ion energy distribution functions, charge-state-resolved ion energy distribution functions of pulsed arc plasmas from Cr and Cr-Al cathodes were recorded with high time resolution by using direct data acquisition from a combined energy and mass analyzer. The authors find increases in intensities of singly charged ions, which is evidence that charge exchange reactions took place in both Cr and Cr-Al systems. In Cr-Al plasmas, the distributions of high-charge-state ions exhibit high energy tails 50 μs after discharge ignition, but no such tails were observed at 500 μs. The energy ratios of ions of different charge states at the beginning of the pulse, when less neutral atoms were in the space in front of the cathode, suggest that ions are accelerated by an electric field. The situation is not so clear after 50 μs due to particle collisions. The initial mean ion charge state of Cr was about the same in Cr and in Cr-Al plasmas, but it decreased more rapidly in Cr-Al plasmas compared to the decay in Cr plasma. The faster decay of the mean ion charge state and ion energy caused by the addition of Al into a pure Cr cathode suggests that the mean ion charge state is determined not only by ionization processes at the cathode spot but also by inelastic collision between different elements

  19. Temporal evolution of ion energy distribution functions and ion charge states of Cr and Cr-Al pulsed arc plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Tanaka, Koichi, E-mail: tanak@mmc.co.jp [Central Research Institute, Mitsubishi Materials Corporation, 1002-14 Mukohyama, Naka-shi, Ibaraki 311-0102 (Japan); Anders, André [Lawrence Berkeley National Laboratory, 1 Cyclotron Road, MS 53, Berkeley, California 94720 (United States)

    2015-11-15

    To study the temporal evolution of ion energy distribution functions, charge-state-resolved ion energy distribution functions of pulsed arc plasmas from Cr and Cr-Al cathodes were recorded with high time resolution by using direct data acquisition from a combined energy and mass analyzer. The authors find increases in intensities of singly charged ions, which is evidence that charge exchange reactions took place in both Cr and Cr-Al systems. In Cr-Al plasmas, the distributions of high-charge-state ions exhibit high energy tails 50 μs after discharge ignition, but no such tails were observed at 500 μs. The energy ratios of ions of different charge states at the beginning of the pulse, when less neutral atoms were in the space in front of the cathode, suggest that ions are accelerated by an electric field. The situation is not so clear after 50 μs due to particle collisions. The initial mean ion charge state of Cr was about the same in Cr and in Cr-Al plasmas, but it decreased more rapidly in Cr-Al plasmas compared to the decay in Cr plasma. The faster decay of the mean ion charge state and ion energy caused by the addition of Al into a pure Cr cathode suggests that the mean ion charge state is determined not only by ionization processes at the cathode spot but also by inelastic collision between different elements.

  20. Low charge state heavy ion production with sub-nanosecond laser.

    Science.gov (United States)

    Kanesue, T; Kumaki, M; Ikeda, S; Okamura, M

    2016-02-01

    We have investigated laser ablation plasma of various species using nanosecond and sub-nanosecond lasers for both high and low charge state ion productions. We found that with sub-nanosecond laser, the generated plasma has a long tail which has low charge state ions determined by an electrostatic ion analyzer even under the laser irradiation condition for highly charged ion production. This can be caused by insufficient laser absorption in plasma plume. This property might be suitable for low charge state ion production. We used a nanosecond laser and a sub-nanosecond laser for low charge state ion production to investigate the difference of generated plasma using the Zirconium target. PMID:26931977

  1. Laser generation of Au ions with charge states above 50(+)

    Czech Academy of Sciences Publication Activity Database

    Láska, Leoš; Jungwirth, Karel; Krása, Josef; Krouský, Eduard; Rohlena, Karel; Skála, Jiří; Velyhan, Andriy; Margarone, D.; Torrisi, L.; Ryc, L.; Ullschmied, Jiří

    2008-01-01

    Roč. 79, - (2008), 02C715/1-02C715/4. ISSN 0034-6748 R&D Projects: GA MŠk(CZ) LC528; GA ČR GA202/05/2475; GA AV ČR IAA100100715 Institutional research plan: CEZ:AV0Z10100523; CEZ:AV0Z20430508 Keywords : laser produced plasma * highly charged Au ions * deconvolution of IC signals Subject RIV: BH - Optics, Masers, Lasers Impact factor: 1.738, year: 2008

  2. Techniques for enhancing the performance of high charge state ECR ion sources

    International Nuclear Information System (INIS)

    Electron Cyclotron Resonance ion source (ECRIS), which produces singly to highly charged ions, is widely used in heavy ion accelerators and is finding applications in industry. It has progressed significantly in recent years thanks to a few techniques, such as multiple-frequency plasma heating, higher mirror magnetic fields and a better cold electron donor. These techniques greatly enhance the production of highly charged ions. More than 1 emA of He2+ and O6+, hundreds of eμA of O7+, Ne8+, Ar12+, more than 100 eμA of intermediate heavy ions with charge states up to Ne9+, Ar13+, Ca13+, Fe13+, Co14+ and Kr18+, tens of eμA of heavy ions with charge states up to Xe28+, Au35+, Bi34+ and U34+ were produced at cw mode operation. At an intensity of about 1 eμA, the charge states for the heavy ions increased up to Xe36+, Au46+, Bi47+ and U48+. More than an order of magnitude enhancement of fully stripped argon ions was achieved (I≥0.1 and h;eμA). Higher charge state ions up to Kr35+, Xe46+ and U64+ at low intensities were produced for the first time from an ECRIS. copyright 1999 American Institute of Physics

  3. Highly Charged Ion Sources

    International Nuclear Information System (INIS)

    In this work a study is made for the factors affecting the production and extraction of highly charged ion beams. Discussion is made for the production of highly charged ions from: the conventional vacuum are ion sources (Pinning PIG and Duoplasmatron DP) and the recent trends type which are (Electron Beam Ion Sources EBIS, Electron Cyclotron Resonance Ion Sources ECRIS and Laser Ion source LIS). The highly charged ions with charge state +7 , O+8 ,Ne+10 , Ar+18 have been extracted from the ECRIS while fully stripped Xe+54 has been extracted from EBIS. Improving the capabilities of the conventional RF ion source to produce multiply charged ions is achieved through the use of electron injection into the plasma or with the use of RF driven ion source. The later is based on coupling the RF power to the discharge through an internal antenna in vacuum are ion source. The argon ion species extracted from these upgraded RF ion sources could reach Ar+5

  4. Charge states of energetic oxygen and sulfur ions in Jupiter's magnetosphere

    Science.gov (United States)

    Clark, G.; Mauk, B. H.; Paranicas, C.; Kollmann, P.; Smith, H. T.

    2016-03-01

    Pitch angle distributions of proton and energetic heavy ion fluxes near Europa's orbit have been measured by the Galileo Energetic Particles Detector (EPD). At similar energies, these distributions have important differences. If their source and transport processes are similar, as we hypothesize here, then it is difficult to reconcile their different pitch angle distributions. By looking at the same question, other researchers have proposed that the heavies are multiply charged, leading to differences in how the particles are lost. This could not be confirmed directly with EPD because that detector does not separate heavy ion measurements by charge state. However, indirect analyses of the data have extracted the charge state of a few sulfur events. We present here a complete list of ion injections observed with EPD over the whole mission. Energetic sulfur and oxygen charge states can be inferred through a dispersion analysis of dynamic injections that makes use of the charge-dependent nature of the gradient-curvature azimuthal drift. We find that sulfur is predominantly multiply charged, whereas oxygen is more evenly distributed between singly and doubly charged states. In addition to current theories on energetic heavy ion transport near the Europa region, we propose that charge gain for the oxygen ions (electron stripping) may play an important role in the character of energetic particles in that region.

  5. Studies of high charge-state ions in the constance B quadrupole mirror

    International Nuclear Information System (INIS)

    Experiments have been initiated into the confinement and extraction physics of high charge-state ions in an ECRH mirror plasma. ECRH mirrors are well suited for producing high Z ions because the hot electron temperature (>100 keV) is sufficient to fully strip heavy ions. The charge state distribution (CSD) of the ion endloss and the ion endloss temperatures have been measured using a time-of-flight analyzer. The CSD of the confined ions has been measured using a VUV spectrometer. Applying ICRH to the plasma was found to lower the Z/sub eff/ of the confined ions while raising the Z/sub eff/ of the extracted ions. The experimental results are compared to theoretical models which include Pastukhov, flow, and spatial-diffusion confinement times. 12 refs., 16 figs

  6. Equilibrium charge state distributions of 14N and 20Ne ions emerging from solids

    International Nuclear Information System (INIS)

    A new technique of backscattering has been developed for the measurement of equilibrium charge state distributions of ions emerging from a solid medium. By this method, equilibrium charge fractions for nitrogen in the energy range from 0.8 to 1.7 MeV and for neon from 1.5 to 4.4 MeV have been measured. The influence of inner shell vacancies produced by violent collisions on the charge state equilibrium is discussed. (Auth.)

  7. Charge state distribution of light ions at glancing collision with solid surface

    International Nuclear Information System (INIS)

    Many experimental results have suggested that the charge state distribution of ions have penetrated through solid is different from that inside the solid. It is important to clarify the physical process taking place at solid surface in order to know the states of ions inside the solid from those observed outside the solid. In the present paper, we report our measurement of charge state distributions of He+ and H2+ ions having been scattered in small angles (less than 40) at surfaces of Au, Ag and C. One of the advantages of the use of the glancing collision of ions at solid surface for the study of ion-surface interaction is that the dwell time of ion near solid surface can be made more than 100 times longer than that in normal transmission experiments. The longer dwell times may alter any contribution of solid surface to electron capture and loss of ions

  8. Performance on the low charge state laser ion source in BNL

    Energy Technology Data Exchange (ETDEWEB)

    Okamura, M.; Alessi, J.; Beebe, E.; Costanzo, M.; DeSanto, L.; Jamilkowski, J.; Kanesue, T.; Lambiase, R.; Lehn, D.; Liaw, C. J.; McCafferty, D.; Morris, J.; Olsen, R.; Pikin, A.; Raparia, D.; Steszyn, A.; Ikeda, S.

    2015-09-07

    On March 2014, a Laser Ion Source (LIS) was commissioned which delivers high-brightness, low-charge-state heavy ions for the hadron accelerator complex in Brookhaven National Laboratory (BNL). Since then, the LIS has provided many heavy ion species successfully. The low-charge-state (mostly singly charged) beams are injected to the Electron Beam Ion Source (EBIS), where ions are then highly ionized to fit to the following accelerator’s Q/M acceptance, like Au32+. Recently we upgraded the LIS to be able to provide two different beams into EBIS on a pulse-to-pulse basis. Now the LIS is simultaneously providing beams for both the Relativistic Heavy Ion Collider (RHIC) and NASA Space Radiation Laboratory (NSRL).

  9. Examination of the charge state distribution of ions in the ECR ion source

    International Nuclear Information System (INIS)

    Complete text of publication follows. The Electron Cyclotron Resonance (ECR) Ion Source of ATOMKI offers the possibility for up-to-date experiments in the field of atomic and plasma physics and for practical applications. Also the methods of the production of highly charged ions are objects of active research. As in the ion source the particles are confined in small volume magnetic traps, the examination without disturbing the plasma is mainly focused on the radiation emitted by them. In the course of our experiments we examine the spectral distribution of x-rays emitted by the plasma of the ECR Ion Source. For the measurements we use a solid state x-ray detector of PIN diode type. With the knowledge of the response function and the efficiency of the detector the recorded spectra can be analyzed and important plasma parameters can be determined from them. During the measurements the detector was situated outside the vacuum chamber so in the course of the analysis also the x-ray transmission of different materials (a 100 μm kapton foil; 25 cm air; 25 μm Be window) had to be taken into account. We recorded x-ray spectra by different settings of the ECRIS and we studied the effects of the tuning parameters on the spectra. In our measurements Ar and Kr gases were used and we analyzed the position of the Kα peak of the working gas incorporating the above detector functions. The shift of the above mentioned peak gives us information on the change of the average ion charge of the plasma. Figure 1 shows a typical x-ray spectrum. We can observe three components in the spectrum: the bremsstrahlung of the electrons, the characteristic lines of the working gas and the characteristic lines of the excited wall materials. X-ray spectrum of Kr ECR plasma and the Change of the energy position of the Kr Kα peak as a function of the power of the microwave field. We plan to continue these measurement using a higher resolution x-ray detector and we will plan to compare the measured

  10. Charge state distribution studies of the metal vapor vacuum arc ion source

    International Nuclear Information System (INIS)

    We have studied the charge state distribution of the ion beam produced by the MEVVA (metal vapor vacuum arc) high current metal ion source. Beams produced from a wide range of cathode materials have been examined and the charge state distributions have been measured as a function of many operational parameters. In this paper we review the charge state data we have accumulated, with particular emphasis on the time history of the distribution throughout the arc current pulse duration. We find that in general the spectra remain quite constant throughout most of the beam pulse, so long as the arc current is constant. There is an interesting early-time transient behavior when the arc is first initiated and the arc current is still rising, during which time the ion charge states produced are observed to be significantly higher than during the steady current region that follows. 12 refs., 5 figs

  11. Charge Breeding of Radioactive Ions

    OpenAIRE

    Wenander, F. J. C.

    2014-01-01

    Charge breeding is a technique to increase the charge state of ions, in many cases radioactive ions. The singly charged radioactive ions, produced in an isotope separator on-line facility, and extracted with a low kinetic energy of some tens of keV, are injected into a charge breeder, where the charge state is increased to Q. The transformed ions are either directed towards a dedicated experiment requiring highly charged ions, or post-accelerated to higher beam energies. In this paper the phy...

  12. Laser Plasmas : Multiple charge states of titanium ions in laser produced plasma

    Indian Academy of Sciences (India)

    M Shukla; S Bandhyopadhyay; V N Rai; A V Kilpio; H C Pant

    2000-11-01

    An intense laser radiation (1012 to 1014 W/cm-2) focused on the solid target creates a hot (≥ 1 keV) and dense plasma having high ionization state. The multiple charged ions with high current densities produced during laser matter interaction have potential application in accelerators as an ion source. This paper presents generation and detection of highly stripped titanium ions (Ti) in laser produced plasma. An Nd:glass laser (KAMETRON) delivering 50 J energy ( = 0.53 m) in 2.5 ns was focused onto a titanium target to produce plasma. This plasma was allowed to drift across a space of ∼ 3 m through a diagnostic hole in the focusing mirror before ions are finally detected with the help of electrostatic ion analyzer. Maximum current density was detected for the charge states of +16 and +17 of Ti ions for laser intensity of ∼ 1014 W/cm-2.

  13. Equilibrium charge-state distributions of highly stripped ions in carbon foils

    International Nuclear Information System (INIS)

    Asymmetric equilibrium charge-state distributions observed for heavy ions (Z approx. >= 7) in carbon foils at high velocities (v > 3.6 x 108 Z0sup(.)45 cm s-1) are closely approximated by a simple statistical distribution: the reduced chi-squared model. The dependences of the mean charge and of the standard deviation of the charge on the projectile velocity are obtained by a previously-known and a newly-proposed relation, respectively. Finally charge-state fractions may be easily predicted using a simple formula depending only on the atomic number and on the velocity of the projectile. (orig.)

  14. Enhanced coulomb counting method for estimating state-of-charge and state-of-health of lithium-ion batteries

    International Nuclear Information System (INIS)

    The coulomb counting method is expedient for state-of-charge (SOC) estimation of lithium-ion batteries with high charging and discharging efficiencies. The charging and discharging characteristics are investigated and reveal that the coulomb counting method is convenient and accurate for estimating the SOC of lithium-ion batteries. A smart estimation method based on coulomb counting is proposed to improve the estimation accuracy. The corrections are made by considering the charging and operating efficiencies. Furthermore, the state-of-health (SOH) is evaluated by the maximum releasable capacity. Through the experiments that emulate practical operations, the SOC estimation method is verified to demonstrate the effectiveness and accuracy.

  15. Recoil ion charge state distribution following the beta(sup +) decay of {sup 21}Na

    Energy Technology Data Exchange (ETDEWEB)

    Scielzo, Nicholas D.; Freedman, Stuart J.; Fujikawa, Brian K.; Vetter, Paul A.

    2003-01-03

    The charge state distribution following the positron decay of 21Na has been measured, with a larger than expected fraction of the daughter 21Ne in positive charge states. No dependence on either the positron or recoil nucleus energy is observed. The data is compared to a simple model based on the sudden approximation. Calculations suggest a small but important contribution from recoil ionization has important consequences for precision beta decay correlation experiments detecting recoil ions.

  16. Recoil ion charge state distribution following the beta(sup +) decay of 21Na

    International Nuclear Information System (INIS)

    The charge state distribution following the positron decay of 21Na has been measured, with a larger than expected fraction of the daughter 21Ne in positive charge states. No dependence on either the positron or recoil nucleus energy is observed. The data is compared to a simple model based on the sudden approximation. Calculations suggest a small but important contribution from recoil ionization has important consequences for precision beta decay correlation experiments detecting recoil ions

  17. The study towards high intensity high charge state laser ion sources

    Science.gov (United States)

    Zhao, H. Y.; Jin, Q. Y.; Sha, S.; Zhang, J. J.; Li, Z. M.; Liu, W.; Sun, L. T.; Zhang, X. Z.; Zhao, H. W.

    2014-02-01

    As one of the candidate ion sources for a planned project, the High Intensity heavy-ion Accelerator Facility, a laser ion source has been being intensively studied at the Institute of Modern Physics in the past two years. The charge state distributions of ions produced by irradiating a pulsed 3 J/8 ns Nd:YAG laser on solid targets of a wide range of elements (C, Al, Ti, Ni, Ag, Ta, and Pb) were measured with an electrostatic ion analyzer spectrometer, which indicates that highly charged ions could be generated from low-to-medium mass elements with the present laser system, while the charge state distributions for high mass elements were relatively low. The shot-to-shot stability of ion pulses was monitored with a Faraday cup for carbon target. The fluctuations within ±2.5% for the peak current and total charge and ±6% for pulse duration were demonstrated with the present setup of the laser ion source, the suppression of which is still possible.

  18. The study towards high intensity high charge state laser ion sources.

    Science.gov (United States)

    Zhao, H Y; Jin, Q Y; Sha, S; Zhang, J J; Li, Z M; Liu, W; Sun, L T; Zhang, X Z; Zhao, H W

    2014-02-01

    As one of the candidate ion sources for a planned project, the High Intensity heavy-ion Accelerator Facility, a laser ion source has been being intensively studied at the Institute of Modern Physics in the past two years. The charge state distributions of ions produced by irradiating a pulsed 3 J/8 ns Nd:YAG laser on solid targets of a wide range of elements (C, Al, Ti, Ni, Ag, Ta, and Pb) were measured with an electrostatic ion analyzer spectrometer, which indicates that highly charged ions could be generated from low-to-medium mass elements with the present laser system, while the charge state distributions for high mass elements were relatively low. The shot-to-shot stability of ion pulses was monitored with a Faraday cup for carbon target. The fluctuations within ±2.5% for the peak current and total charge and ±6% for pulse duration were demonstrated with the present setup of the laser ion source, the suppression of which is still possible. PMID:24593615

  19. High charge state carbon and oxygen ions in Earth's equatorial quasi-trapping region

    Science.gov (United States)

    Christon, S. P.; Hamilton, D. C.; Gloeckler, G.; Eastmann, T. E.

    1994-01-01

    Observations of energetic (1.5 - 300 keV/e) medium-to-high charge state (+3 less than or equal to Q less than or equal to +7) solar wind origin C and O ions made in the quasi-trapping region (QTR) of Earth's magnetosphere are compared to ion trajectories calculated in model equatorial magnetospheric magnetic and electric fields. These comparisons indicate that solar wind ions entering the QTR on the nightside as an energetic component of the plasma sheet exit the region on the dayside, experiencing little or no charge exchange on the way. Measurements made by the CHarge Energy Mass (CHEM) ion spectrometer on board the Active Magnetospheric Particle Tracer Explorer/Charge Composition Explorer (AMPTE/CCE) spacecraft at 7 less than L less than 9 from September 1984 to January 1989 are the source of the new results contained herein: quantitative long-term determination of number densities, average energies, energy spectra, local time distributions, and their variation with geomagnetic disturbance level as indexed by Kp. Solar wind primaries (ions with charge states unchanged) and their secondaries (ions with generally lower charge states produced from primaries in the magnetosphere via charge exchange)are observed throughout the QTR and have distinctly different local time variations that persist over the entire 4-year analysis interval. During Kp larger than or equal to 3 deg intervals, primary ion (e.g., O(+6)) densities exhibit a pronounced predawn maximum with average energy minimum and a broad near-local-noon density minimum with average energy maximum. Secondary ion (e.g., O(+5)) densities do not have an identifiable predawn peak, rather they have a broad dayside maximum peaked in local morning and a nightside minimum. During Kp less than or equal to 2(-) intervals, primary ion density peaks are less intense, broader in local time extent, and centered near midnight, while secondary ion density local time variations diminish. The long-time-interval baseline helps

  20. Dependence of multiply charged ions on the polarization state in nanosecond laser-benzene cluster interaction

    Science.gov (United States)

    Wang, Weiguo; Zhao, Wuduo; Hua, Lei; Hou, Keyong; Li, Haiyang

    2016-05-01

    This paper investigated the dependence of multiply charged ions on the laser polarization state when benzene cluster was irradiated with 532 and 1064 nm nanosecond laser. A circle, square and flower distribution for C2+, C3+ and C4+ were observed with 532 nm laser respectively, while flower petals for C2+, C3+ and C4+ were observed at 1064 nm as the laser polarization varied. A theoretical calculation was performed to interpret the polarization state and wavelength dependence of the multiply charged ions. The simulated results agreed well with the experimental observation with considering the contribution from the cluster disintegration.

  1. Determination of charge state characteristics of selected scattered ions using a multiple thin film detector arrangement

    International Nuclear Information System (INIS)

    A nuclear charged particle detector has been designed which consists of a stack of three Thin Film Detectors (TFD), measuring the specific luminescence of the transiting ion, and a terminal surface barrier detector measuring the residual energy. To test the response of this detector, an experiment was performed in which several isotopes of germanium and selenium were scattered off a gold target and collimated through the detector assembly. The energies of the scattered ions ranged from 0.65 MeV/amu to 2 MeV/amu, bracketing the peak of the stopping power curve of the ions. An improved nuclear charge resolution is seen when using the multiple TFD arrangement. The analysis of the data also shows new information on the characteristics of the charge states of the ions scattered in small impact parameter collisions with the gold target nuclei

  2. Charge states distribution of 3350 keV He ions channeled in silicon

    CERN Document Server

    Bentini, G G; Bianconi, M; Lotti, R; Lulli, G

    2002-01-01

    When an ion beam is aligned along a major crystalline axis the dominant interaction is with valence electrons. In this condition the charge exchange processes mostly concern the interaction between the incident ion and a quasi-free electron gas and a strong reduction of the charge-changing probabilities is expected. In this work, 3350 keV He sup + and He sup 2 sup + ions were aligned at small tilt angles about the axis of a 4650 A silicon crystalline membrane. The charge state distribution (CSD) of the transmitted ions was detected by an electro-magnetic analyzer having a very small acceptance angle. In these conditions the equilibration of the CSD was not yet reached and this allowed, making use of simple approximations, for the measurement of the valence electron loss cross-section.

  3. Heavy ion charge-state distribution effects on energy loss in plasmas

    Science.gov (United States)

    Barriga-Carrasco, Manuel D.

    2013-10-01

    According to dielectric formalism, the energy loss of the heavy ion depends on its velocity and its charge density. Also, it depends on the target through its dielectric function; here the random phase approximation is used because it correctly describes fully ionized plasmas at any degeneracy. On the other hand, the Brandt-Kitagawa (BK) model is employed to depict the projectile charge space distribution, and the stripping criterion of Kreussler is used to determine its mean charge state . This latter criterion implies that the mean charge state depends on the electron density and temperature of the plasma. Also, the initial charge state of the heavy ion is crucial for calculating inside the plasma. Comparing our models and estimations with experimental data, a very good agreement is found. It is noticed that the energy loss in plasmas is higher than that in the same cold gas cases, confirming the well-known enhanced plasma stopping (EPS). In this case, EPS is only due to the increase in projectile effective charge Qeff, which is obtained as the ratio between the energy loss of each heavy ion and that of the proton in the same plasma conditions. The ratio between the effective charges in plasmas and in cold gases is higher than 1, but it is not as high as thought in the past. Finally, another significant issue is that the calculated effective charge in plasmas Qeff is greater than the mean charge state , which is due to the incorporation of the BK charge distribution. When estimations are performed without this distribution, they do not fit well with experimental data.

  4. Inline state of health estimation of lithium-ion batteries using state of charge calculation

    Science.gov (United States)

    Sepasi, Saeed; Ghorbani, Reza; Liaw, Bor Yann

    2015-12-01

    The determination of state-of-health (SOH) and state-of-charge (SOC) is challenging and remains as an active research area in academia and industry due to its importance for Li-ion battery applications. The estimation process poses more challenges after substantial battery aging. This paper presents an inline SOH and SOC estimation method for Li-ion battery packs, specifically for those based on LiFePO4 chemistry. This new hybridized SOC and SOH estimator can be used for battery packs. Inline estimated model parameters were used in a compounded SOC + SOH estimator consisting of the SOC calculation based on coulomb counting method as an expedient approach and an SOH observer using an extended Kalman filter (EKF) technique for calibrating the estimates from the coulomb counting method. The algorithm's low SOC and SOH estimation error, fast response time, and less-demanding computational requirement make it practical for on-board estimations. The simulation and experimental results, along with the test bed structure, are presented to validate the proposed methodology on a single cell and a 3S1P LiFePO4 battery pack.

  5. The average equilibrium charge-states of heavy ions with Z > 60 stripped in He and H2

    International Nuclear Information System (INIS)

    The equilibrium charges of heavy ions (61 < Z < 101) with energies from 5 to 100 MeV stripped in He and H2 have been measured. New empirical formulae for the average charge state are presented. (orig.)

  6. Charge-state-dependent energy loss of slow ions. II. Statistical atom model

    Science.gov (United States)

    Wilhelm, Richard A.; Möller, Wolfhard

    2016-05-01

    A model for charge-dependent energy loss of slow ions is developed based on the Thomas-Fermi statistical model of atoms. Using a modified electrostatic potential which takes the ionic charge into account, nuclear and electronic energy transfers are calculated, the latter by an extension of the Firsov model. To evaluate the importance of multiple collisions even in nanometer-thick target materials we use the charge-state-dependent potentials in a Monte Carlo simulation in the binary collision approximation and compare the results to experiment. The Monte Carlo results reproduce the incident charge-state dependence of measured data well [see R. A. Wilhelm et al., Phys. Rev. A 93, 052708 (2016), 10.1103/PhysRevA.93.052708], even though the experimentally observed charge exchange dependence is not included in the model.

  7. Ion charge state distributions of pulsed vacuum arc plasmas in strong magnetic fields

    International Nuclear Information System (INIS)

    Vacuum arc plasmas with discharge currents of 300 A and duration 250 μs have been produced in strong magnetic fields up to 4 T. Ion charge state distributions have been measured for C, Al, Ag, Ta, Pt, Ho, and Er with a time-of-flight charge-mass spectrometer. Our previous measurements have been confirmed which show that ion charge states can be considerably enhanced when increasing the magnetic field up to about 1 T. The new measurements address the question of whether or not the additional increase continues at even higher magnetic field strength. It has been found that the increase becomes insignificant for field strengths greater than 1 T. Ion charge state distributions are almost constant for magnetic field strengths between 2 and 4 T. The results are explained by comparing the free expansion length with the freezing length. The most significant changes of charge state distributions are observed when these lengths are similar. copyright 1998 American Institute of Physics

  8. Ion charge state distributions of pulsed vacuum arc plasmas in strong magnetic fields

    International Nuclear Information System (INIS)

    Vacuum arc plasmas with discharge currents of 300 A and duration 250 μs have been produced in strong magnetic fields up to 4 T. Ion charge state distributions have been measured for C, Al, Ag, Ta, Pt, Ho, and Er with a time-of-flight charge-mass-spectrometer. Our previous measurements have been confirmed which show that ion charge states can be considerably enhanced when increasing the magnetic field up to about 1 T. The new measurements address the question of whether or not the additional increase continues at even higher magnetic field strength. It has been found that the increase becomes insignificant for field strengths greater than 1 T. Ion charge state distributions are almost constant for magnetic field strengths between 2 and 4 T. The results are explained by comparing the free expansion length with the freezing length. The most significant changes of charge state distributions are observed when these lengths are similar. copyright 1998 American Institute of Physics

  9. Charge-state dependence of electron loss from H by collisions with heavy, highly stripped ions

    International Nuclear Information System (INIS)

    Theoretical calculations, confirmed by experimental measurements, are used to obtain a new scaling for electron loss from a hydrogen atom in collision with a heavy, highly stripped ion. The calculations cover the energy range 50 to 5000 keV/amu and charge states q from 1 to 50. The experiments are in the range 108 to 1140 keV/amu and charge states 3 to 22. A simple analytic expression that describes the electron-loss cross section for 1 < or = q < or = 50 in the energy range 50 to 5000 keV/amu is presented

  10. Calculation of Ion Charge State Distributions After Inner-Shell Ionization in Xe Atom

    International Nuclear Information System (INIS)

    The vacancy cascades following initial inner-shell vacancies in single and multi-ionized atoms often lead to highly charged residual ions. The inner-shell vacancy produced by ionization processes may decay by either a radiative or non-radiative transition. In addition to the vacancy filling processes, there is an electron shake off process due to the change of core potential of the atom. In the calculation of vacancy cascades, the radiative (x-ray) and non-radiative (Auger and Coster-Kronig) branching ratios give valuable information on the de-excitation dynamics of an atom with inner-shell vacancy. The production of multi-charged ions yield by the Auger cascades following inner shell ionization of an atom has been studied both experimentally and theoretically. Multi-charged Xe ions following de-excitation of K-, L1-, L2,3-, M1-, M2,3- and M4,5 subshell vacancies are calculated using Monte-Carlo algorithm to simulate the vacancy cascade development. Fluorescence yield (radiative) and Auger, Coster- Kronig yield (non- radiative) are evaluated. The decay of K hole state through radiative transitions is found to be more probable than non-radiative transitions in the first step of de-excitation. On the other hand, the decay of L, M vacancies through non-radiative transitions are more probable. The K shell ionization in Xe atom mainly yields Xe7+, Xe8+, Xe9+ and Xe10+ ions, and the charged X8+ ions are the highest. The main product from the L1- shell ionization is found to be Xe8+, Xe9+ ions, while the charged Xe8+ ions predominate at L2,3 hole states. The charged Xe6+, Xe7+ and Xe8+ ions mainly yield from 3s1/2 and 3p1/2,3/2 ionization, while Xe in 3d3/2,5/2 hole states mainly turns into Xe4+ and Xe5+ ions. The present results are found to agree well with the experimental data.

  11. Calculation of Ion Charge State Distributions After Inner-Shell Ionization in Xe Atom

    International Nuclear Information System (INIS)

    The vacancy cascades following initial inner-shell vacancies in single and multi-ionized atoms often lead to highly charged residual ions. The inner-shell vacancy produced by ionization processes may decay by either a radiative or non-radiative transition. In addition to the vacancy filling processes, there is an electron shake off process due to the change of core potential of the atom. In the calculation of vacancy cascades, the radiative (x-ray) and non-radiative (Auger and Coster-Kronig) branching ratios give valuable information on the de-excitation dynamics of an atom with inner-shell vacancy. The production of multi-charged ions yield by the Auger cascades following inner shell ionization of an atom has been studied both experimentally and theoretically. Multi-charged Xe ions following de-excitation of K, L1, L2,3, M1, M2,3 and M4,5 subshell vacancies are calculated using Monte-Carlo algorithm to simulate the vacancy cascade development. Fluorescence yield (radiative) and Auger, Coster- Kronig yield (non- radiative) are evaluated. The decay of K hole state through radiative transitions is found to be more probable than non-radiative transitions in the first step of de-excitation. On the other hand, the decay of L, M vacancies through non-radiative transitions are more probable. The K shell ionization in Xe atom mainly yields Xe7+, Xe8+, Xe9+ and Xe10+ ions, and the charged X8+ ions are the highest. The main product from the L1 shell ionization is found to be Xe8+, Xe9+ ions, while the charged Xe8+ ions predominate at L2,3 hole states. The charged Xe6+, Xe7+ and Xe8+ ions mainly yield from 3s1/2 and 3p1/2,3/2 ionization, while Xe in 3d3/2,5/2 hole states mainly turns into Xe4+ and Xe5+ ions. The present results are found to agree well with the experimental data. (author)

  12. Charge Breeding of Radioactive Ions

    CERN Document Server

    Wenander, F J C

    2013-01-01

    Charge breeding is a technique to increase the charge state of ions, in many cases radioactive ions. The singly charged radioactive ions, produced in an isotope separator on-line facility, and extracted with a low kinetic energy of some tens of keV, are injected into a charge breeder, where the charge state is increased to Q. The transformed ions are either directed towards a dedicated experiment requiring highly charged ions, or post-accelerated to higher beam energies. In this paper the physics processes involved in the production of highly charged ions will be introduced, and the injection and extraction beam parameters of the charge breeder defined. A description of the three main charge-breeding methods is given, namely: electron stripping in gas jet or foil; external ion injection into an electron-beam ion source/trap (EBIS/T); and external ion injection into an electron cyclotron resonance ion source (ECRIS). In addition, some preparatory devices for charge breeding and practical beam delivery aspects ...

  13. The evolution of ion charge states in cathodic vacuum arc plasmas: a review

    Energy Technology Data Exchange (ETDEWEB)

    Anders, Andre

    2011-12-18

    Cathodic vacuum arc plasmas are known to contain multiply charged ions. 20 years after “Pressure Ionization: its role in metal vapour vacuum arc plasmas and ion sources” appeared in vol. 1 of Plasma Sources Science and Technology, it is a great opportunity to re-visit the issue of pressure ionization, a non-ideal plasma effect, and put it in perspective to the many other factors that influence observable charge state distributions, such as the role of the cathode material, the path in the density-temperature phase diagram, the “noise” in vacuum arc plasma as described by a fractal model approach, the effects of external magnetic fields and charge exchange collisions with neutrals. A much more complex image of the vacuum arc plasma emerges putting decades of experimentation and modeling in perspective.

  14. High intensity high charge state ion beam production with an evaporative cooling magnet ECRIS

    Energy Technology Data Exchange (ETDEWEB)

    Lu, W., E-mail: luwang@impcas.ac.cn; Qian, C.; Sun, L. T.; Zhang, X. Z.; Feng, Y. C.; Ma, B. H.; Zhao, H. W.; Zhan, W. L. [Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 73000 (China); Fang, X.; Guo, J. W.; Yang, Y. [Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 73000 (China); University of Chinese Academy of Sciences, Beijing 100049 (China); Xiong, B.; Ruan, L. [Institute of Electrical Engineering, CAS, Beijing 100190 (China); Xie, D. [Nuclear Science Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States)

    2016-02-15

    LECR4 (Lanzhou ECR ion source No. 4) is a room temperature electron cyclotron resonance ion source, designed to produce high current, high charge state ion beams for the SSC-LINAC injector (a new injector for sector separated cyclotron) at the Institute of Modern Physics. LECR4 also serves as a PoP machine for the application of evaporative cooling technology in accelerator field. To achieve those goals, LECR4 ECR ion source has been optimized for the operation at 18 GHz. During 2014, LECR4 ion source was commissioned at 18 GHz microwave of 1.6 kW. To further study the influence of injection stage to the production of medium and high charge state ion beams, in March 2015, the injection stage with pumping system was installed, and some optimum results were produced, such as 560 eμA of O{sup 7+}, 620 eμA of Ar{sup 11+}, 430 eμA of Ar{sup 12+}, 430 eμA of Xe{sup 20+}, and so on. The comparison will be discussed in the paper.

  15. High intensity high charge state ion beam production with an evaporative cooling magnet ECRIS

    International Nuclear Information System (INIS)

    LECR4 (Lanzhou ECR ion source No. 4) is a room temperature electron cyclotron resonance ion source, designed to produce high current, high charge state ion beams for the SSC-LINAC injector (a new injector for sector separated cyclotron) at the Institute of Modern Physics. LECR4 also serves as a PoP machine for the application of evaporative cooling technology in accelerator field. To achieve those goals, LECR4 ECR ion source has been optimized for the operation at 18 GHz. During 2014, LECR4 ion source was commissioned at 18 GHz microwave of 1.6 kW. To further study the influence of injection stage to the production of medium and high charge state ion beams, in March 2015, the injection stage with pumping system was installed, and some optimum results were produced, such as 560 eμA of O7+, 620 eμA of Ar11+, 430 eμA of Ar12+, 430 eμA of Xe20+, and so on. The comparison will be discussed in the paper

  16. High intensity high charge state ion beam production with an evaporative cooling magnet ECRIS

    Science.gov (United States)

    Lu, W.; Qian, C.; Sun, L. T.; Zhang, X. Z.; Fang, X.; Guo, J. W.; Yang, Y.; Feng, Y. C.; Ma, B. H.; Xiong, B.; Ruan, L.; Zhao, H. W.; Zhan, W. L.; Xie, D.

    2016-02-01

    LECR4 (Lanzhou ECR ion source No. 4) is a room temperature electron cyclotron resonance ion source, designed to produce high current, high charge state ion beams for the SSC-LINAC injector (a new injector for sector separated cyclotron) at the Institute of Modern Physics. LECR4 also serves as a PoP machine for the application of evaporative cooling technology in accelerator field. To achieve those goals, LECR4 ECR ion source has been optimized for the operation at 18 GHz. During 2014, LECR4 ion source was commissioned at 18 GHz microwave of 1.6 kW. To further study the influence of injection stage to the production of medium and high charge state ion beams, in March 2015, the injection stage with pumping system was installed, and some optimum results were produced, such as 560 eμA of O7+, 620 eμA of Ar11+, 430 eμA of Ar12+, 430 eμA of Xe20+, and so on. The comparison will be discussed in the paper.

  17. Energy loss and charge state distribution of calcium ions in dense moderately coupled carbon plasma

    International Nuclear Information System (INIS)

    In this thesis the interaction of swift calcium ions (Energy: 3.5 MeV/u) with a dense and moderately coupled carbon plasma (Coupling parameter: Γ=0.1-0.5) is investigated. The plasma state is generated by heating a thin carbon foil volumetrically by thermal X-ray radiation. The thermal X-ray radiation itself is generated by the conversion of a high energy laser beam in a hohlraum cavity. Compared to earlier ion stopping experiments the electron density and the plasma coupling parameter could be increased by an order of magnitude. This work provides the first time experimental energy loss and charge state distribution data in this moderately coupled interaction regime. The thesis consists of a theoretical part where the ion beam plasma interaction is studied for a broad range of plasma parameters and an experimental part where the ion beam interaction with the hohlraum plasma target is measured. All the described experiments were carried out at the GSI Helmholtzzentrum fuer Schwerionenforschung in Darmstadt. This facility offers the unique possibility to combine a heavy ion beam from an accelerator with a high energy laser beam in one interaction chamber. An intense laser pulse (150 J of laser energy in 1 ns at λL=527 nm) is focused inside a 600 μm diameter spherical cavity and generates a hot gold plasma that emits X-rays. The absorbed and reemitted radiation establishes a spatially uniform temperature distribution in the cavity and serves as an intense, isotropic X-ray source with a quasi-thermal spectral distribution. These thermal X-rays with a radiation temperature of Tr=98±6 eV then propagate into a secondary cylindrical hohlraum (diameter: 1000 μm, length: 950 μm) where they volumetrically heat two thin carbon foils to the plasma state. The radiation temperature in the secondary hohlraum is Tr=33±5 eV. This indirect laser heating scheme has the advantage that the whole sample volume is instantaneously heated and that the plasma is inertially and

  18. Design of a CW high charge state heavy ion RFQ for SSC-LINAC

    International Nuclear Information System (INIS)

    The new linac injector SSC-LINAC has been proposed to replace the existing Separator Sector Cyclotron (SSC). This effort is to improve the beam efficiency of the Heavy Ion Research Facility of Lanzhou (HIRFL). As a key component of the linac, a continuous-wave (CW) mode high charge state heavy ion radio-frequency quadrupole (RFQ) accelerator has been designed. It accelerates ions with the ratio of mass to charge up to 7 from 3.728 keV/u to 143 keV/u. The requirements of CW mode operation and the transportation of intense beam have been considered as the greatest challenges. The design is based on 238U34+ beams, whose current is 0.5 pmA (0.5 particle mili-ampere, which is the measured 17 emA electric current divided by charge state of heavy ions). It achieves the transmission efficiency of 94% with 2508.46 mm long vanes in simulation. To improve the transmission efficiency and quality of the beams, the phase advance has been taken into account to analyze the reasons of beam loss and emittance growth. Parametric resonance and beam mismatch have been carefully avoided by adjusting the structure parameters. The parameter-sensitivity of the design is checked by transportation simulations of various input beams. To verify the applicability of machining, the effects of different vane manufacturing methods on beam dynamics are presented in this paper.

  19. Axial ion charge state distribution in the vacuum arc plasma jet

    International Nuclear Information System (INIS)

    We report on our experimental studies of the ion charge state distribution (CSD) of vacuum arc plasmas using a time-of-flight diagnostic method. The dependence of the CSD on the axial distance from the plasma source region was measured for a titanium vacuum arc. It was found that the axial CSD profile is nonuniform. Generally, the mean charge state increases approximately linearly with axial distance from about 1.7 at 12 cm up to 1.9 at 25 cm from the plasma source. A model for ion transport in the free boundary plasma jet is proposed which is based on the existence of an electric field in the quasineutral plasma. This model qualitatively explains the experimental results. (c) 2000 American Institute of Physics

  20. Charge state and energy loss of relativistic heavy ions in matter

    International Nuclear Information System (INIS)

    Relativistic heavy-ion collisions of few-electron projectiles ranging from argon up to uranium have been investigated in solid and gaseous media. Electron-loss and electron-capture cross sections, charge-state distributions, as well as energy loss and energy deposition have been measured and are compared with theoretical predictions. Especially fully-ionized heavy projectiles represent a unique possibility to test atomic-collision theories. (orig.)

  1. Influence of argon and oxygen on charge-state-resolved ion energy distributions of filtered aluminum arcs

    OpenAIRE

    Rosen, Johanna; Anders, Andre; Mraz, Stanislav; Atiser, Adil; Schneider, Jochen M.

    2006-01-01

    The charge-state-resolved ion energy distributions (IEDs) in filtered aluminum vacuum arc plasmas were measured and analyzed at different oxygen and argon pressures in the range 0.5 8.0 mTorr. A significant reduction of the ion energy was detected as the pressure was increased, most pronounced in an argon environment and for the higher charge states. The corresponding average charge state decreased from 1.87 to 1.0 with increasing pressure. The IEDs of all metal ions in oxygen were fitte...

  2. A compact electron beam ion source with integrated Wien filter providing mass and charge state separated beams of highly charged ions

    International Nuclear Information System (INIS)

    A Wien filter was designed for and tested with a room temperature electron beam ion source (EBIS). Xenon charge state spectra up to the charge state Xe46+ were resolved as well as the isotopes of krypton using apertures of different sizes. The complete setup consisting of an EBIS and a Wien filter has a length of less than 1 m substituting a complete classical beamline setup. The Wien filter is equipped with removable permanent magnets. Hence total beam current measurements are possible via simple removal of the permanent magnets. In dependence on the needs of resolution a weak (0.2 T) or a strong (0.5 T) magnets setup can be used. In this paper the principle of operation and the design of the Wien filter meeting the requirements of an EBIS are briefly discussed. The first ion beam extraction and separation experiments with a Dresden EBIS are presented.

  3. A compact electron beam ion source with integrated Wien filter providing mass and charge state separated beams of highly charged ions.

    Science.gov (United States)

    Schmidt, M; Peng, H; Zschornack, G; Sykora, S

    2009-06-01

    A Wien filter was designed for and tested with a room temperature electron beam ion source (EBIS). Xenon charge state spectra up to the charge state Xe46+ were resolved as well as the isotopes of krypton using apertures of different sizes. The complete setup consisting of an EBIS and a Wien filter has a length of less than 1 m substituting a complete classical beamline setup. The Wien filter is equipped with removable permanent magnets. Hence total beam current measurements are possible via simple removal of the permanent magnets. In dependence on the needs of resolution a weak (0.2 T) or a strong (0.5 T) magnets setup can be used. In this paper the principle of operation and the design of the Wien filter meeting the requirements of an EBIS are briefly discussed. The first ion beam extraction and separation experiments with a Dresden EBIS are presented. PMID:19566197

  4. Ion charge state distributions of vacuum arc plasmas: The origin of species

    International Nuclear Information System (INIS)

    Vacuum arc plasmas are produced at micrometer-size, nonstationary cathode spots. Ion charge state distributions (CSD close-quote s) are experimentally known for 50 elements, but the theoretical understanding is unsatisfactory. In this paper, CSD close-quote s of vacuum arc plasmas are calculated under the assumption that the spot plasma experiences an instantaneous transition from equilibrium to nonequilibrium while expanding. Observable charge state distributions are the result of a freezing process at this transition. open-quotes Frozenclose quotes CSD close-quote s have been calculated using Saha equations in the Debye-Hueckel approximation of the nonideal plasma for all metals of the Periodic Table and for boron, carbon, silicon, and germanium. The results are presented in a open-quotes periodic table of CSD.close quotes The table contains also the mean ion charge state, the neutral vapor fraction, and the effective plasma temperature and density at the freezing point for each element. The validity of the concepts of open-quotes instantaneous freezingclose quotes and open-quotes effective temperature and densityclose quotes is discussed for low and high currents and for the presence of a magnetic field. Temperature fluctuations have been identified to cause broadening of CSD close-quote s. copyright 1997 The American Physical Society

  5. Heavy Inertial Confinement Energy: Interactions Involoving Low charge State Heavy Ion Injection Beams

    Energy Technology Data Exchange (ETDEWEB)

    DuBois, Robert D

    2006-04-14

    During the contract period, absolute cross sections for projectile ionization, and in some cases for target ionization, were measured for energetic (MeV/u) low-charge-state heavy ions interacting with gases typically found in high and ultra-high vacuum environments. This information is of interest to high-energy-density research projects as inelastic interactions with background gases can lead to serious detrimental effects when intense ion beams are accelerated to high energies, transported and possibly confined in storage rings. Thus this research impacts research and design parameters associated with projects such as the Heavy Ion Fusion Project, the High Current and Integrated Beam Experiments in the USA and the accelerator upgrade at GSI-Darmstadt, Germany. Via collaborative studies performed at GSI-Darmstadt, at the University of East Carolina, and Texas A&M University, absolute cross sections were measured for a series of collision systems using MeV/u heavy ions possessing most, or nearly all, of their bound electrons, e.g., 1.4 MeV/u Ar{sup +}, Xe{sup 3+}, and U{sup 4,6,10+}. Interactions involving such low-charge-state heavy ions at such high energies had never been previously explored. Using these, and data taken from the literature, an empirical model was developed for extrapolation to much higher energies. In order to extend our measurements to much higher energies, the gas target at the Experimental Storage Ring in GSI-Darmstadt was used. Cross sections were measured between 20 and 50 MeV/u for U{sup 28+}- H{sub 2} and - N{sub 2}, the primary components found in high and ultra-high vacuum systems. Storage lifetime measurements, information inversely proportional to the cross section, were performed up to 180 MeV/u. The lifetime and cross section data test various theoretical approaches used to calculate cross sections for many-electron systems. Various high energy density research projects directly benefit by this information. As a result, the general

  6. Adding high time resolution to charge-state-specific ion energy measurements for pulsed copper vacuum arc plasmas

    CERN Document Server

    Tanaka, Koichi; Zhou, Xue; Anders, André

    2015-01-01

    Charge-state-resolved ion energy-time-distributions of pulsed Cu arc plasma were obtained by using direct (time dependent) acquisition of the ion detection signal from a commercial ion mass-per-charge and energy-per-charge analyzer. We find a shift of energies of Cu2+, Cu3+ and Cu4+ ions to lower values during the first few hundred microseconds after arc ignition, which is evidence for particle collisions in the plasma. The generation of Cu1+ ions in the later part of the pulse, measured by the increase of Cu1+ signal intensity and an associated slight reduction of the mean charge state point to charge exchange reactions between ions and neutrals. At the very beginning of the pulse, when the plasma expands into vacuum and the plasma potential strongly fluctuates, ions with much higher energy (over 200 eV) were observed. Early in the pulse, the ion energies observed are approximately proportional to the ion charge state, and we conclude that the acceleration mechanism is primarily based on acceleration in an e...

  7. Bound state properties and photodetachment of the negatively charged hydrogen ions

    OpenAIRE

    Frolov, Alexei M.

    2015-01-01

    Absorption of infrared and visible radiation from stellar emission spectra by the negatively charged hydrogen ions H$^{-}$ is considered. The explicit formula for the photodetachment cross-section of the negatively charged hydrogen ion(s) is derived. Photodetachemnt cross-sections of the ${}^{\\infty}$H$^{-}$, ${}^{3}$H$^{-}$ (or T$^{-}$), ${}^{2}$H$^{-}$ (or D$^{-}$) and ${}^{1}$H$^{-}$ ions are determined to high accuracy and for a large number of photo-electron momenta/energies. We introduc...

  8. State-Of-Charge Estimation of Li-Ion Battery Using Extended Kalman Filter

    Directory of Open Access Journals (Sweden)

    Feng Jin

    2013-07-01

    Full Text Available The Li-ion battery is studied base on its equivalent circuit PNGV model. The model parameters are identified by HPPC test. The discrete state space equation is established according to the model. The basic theory of extended Kalman filter algorithm is studied and then the filtering algorithm is set up under the noisy environments. Finally, a kind of electric car is used for testing under the UDDS driving condition. The difference between the simulation value using extended Kalman filter under the noisy environment and the theoretical value is compared. The result indicated that the extended Kalman filter keeps an excellent precision in state of charge estimation of Li-ion battery and performs well when disturbance happens.

  9. Observations of energetic oxygen and carbon ions with charge states between 3 and 6 in the magnetosphere

    Science.gov (United States)

    Kremser, G.; Stuedemann, W.; Wilken, B.; Gloeckler, G.; Hamilton, D. C.

    1988-01-01

    Data obtained by the AMPTE/CCE charge-energy-mass spectrometer are used to study the average spatial distributions of oxygen and carbon ions with charge states between 3 and 6. The O(6+) and C(6+) ion fluxes are found to increase with the drift shell parameter L up to a constant level at L of not less than 7. It is suggested that the diurnal variations noted are related to the shape of the L profiles. The results support a model in which the solar wind origin O(6+) and C(6+) ions and the terrestrial origin O(+) and O(2+) ions are transported from the tail towards the earth. Charge exchange processes near the earth produce the oxygen and carbon ions with charge states between 3 and 5.

  10. Energy and charge state dependences of transfer ionization to single capture ratio for fast multiply charged ions on helium

    Science.gov (United States)

    Unal, Ridvan

    The charge state and energy dependences of Transfer Ionization (TI) and Single Capture (SC) processes in collisions of multiply charged ions with He from intermediate to high velocities are investigated using coincident recoil ion momentum spectroscopy. The collision chamber is commissioned on the 15-degree port of a switching magnet, which allows the delivery of a beam with very little impurity. The target was provided from a supersonic He jet with a two-stage collimation. The two-stage, geometrically cooled, supersonic He jet has significantly reduced background contribution to the spectrum compared to a single stage He jet. In the case of a differentially pumped gas cell complex calculations based on assumptions for the correction due to the collisions with the contaminant beam led to corrections, which were up to 50%. The new setup allows one to make a direct separation of contaminant processes in the experimental data using the longitudinal momentum spectra. Furthermore, this correction is much smaller (about 8.8%) yielding better overall precision. The collision systems reported here are 1 MeV/u O(4--8)+ , 0.5--2.5 MeV/u F(4--9)+, 2.0 MeV/u Ti 15,17,18+, 1.6--1.75 MeV/u Cu18,20+ and 0.25--0.5 MeV/u I(15--25)+ ions interacting with helium. We have determined the sTIsSC ratio for high velocity highly charged ions on He at velocities in the range of 6 to 10 au and observed that the ratio is monotonically decreasing with velocity. Furthermore, we see a ratio that follows a q2 dependence up to approximately q = 9. Above q = 9 the experimental values exceed the q2 dependence prediction due to antiscreening. C. D. Lin and H. C. Tseng have performed coupled channel calculations for the energy dependence of TI and SC for F9+ + He and find values slightly higher than our measured values, but with approximately the same energy dependence. The new data, Si, Ti and Cu, go up only to q = 20 and show a smooth monotonically increasing TI/SC ratio. The TI/SC ratio for I (15

  11. Energy-dependent Charge States and Their Connection with Ion Abundances in Impulsive Solar Energetic Particle Events

    Science.gov (United States)

    DiFabio, R.; Guo, Z.; Möbius, E.; Klecker, B.; Kucharek, H.; Mason, G. M.; Popecki, M.

    2008-11-01

    Impulsive solar energetic particle (SEP) events show substantial enhancements of heavy ions and 3He over the composition in the Sun's atmosphere. Mass per charge dependent acceleration mechanisms have been proposed to account for this preferential acceleration. However, a problem emerged for all the preferential acceleration models with the measurement of ionization states near 1 MeV nucleon-1, which showed that ions from C to Mg are fully stripped, a challenge that had been recognized early on. Since all models relied on differences in the charge-to-mass ratio to enable preferential acceleration, the proposed mechanisms were incompatible with this observation. Recent observations of the ionic charge states at lower energies have revealed a dependence on energy, with the charge states decreasing for lower energy ions. This raises the possibility that the low-energy charge states reflect the plasma conditions at the acceleration site, while the high-energy charge states are due to stripping low in the solar corona. In a survey of impulsive events we show that the increase of the Fe charge states with energy is highly significant for the sample of events and thus most likely a general feature of impulsive events. To see whether there is a connection between the enhancements and charge states, we extended the ACE SEPICA charge-state observations to lower energies and combined them with the ion fluxes from ACE ULEIS for impulsive events observed between 1997 and 2000. We find a positive correlation between the abundance ratios and the charge states at low energy, while the charge states at the highest energy do not demonstrate such dependence. This supports the idea that the higher mass particles are preferentially accelerated before being stripped.

  12. Evaluation of Model Based State of Charge Estimation Methods for Lithium-Ion Batteries

    Directory of Open Access Journals (Sweden)

    Zhongyue Zou

    2014-08-01

    Full Text Available Four model-based State of Charge (SOC estimation methods for lithium-ion (Li-ion batteries are studied and evaluated in this paper. Different from existing literatures, this work evaluates different aspects of the SOC estimation, such as the estimation error distribution, the estimation rise time, the estimation time consumption, etc. The equivalent model of the battery is introduced and the state function of the model is deduced. The four model-based SOC estimation methods are analyzed first. Simulations and experiments are then established to evaluate the four methods. The urban dynamometer driving schedule (UDDS current profiles are applied to simulate the drive situations of an electrified vehicle, and a genetic algorithm is utilized to identify the model parameters to find the optimal parameters of the model of the Li-ion battery. The simulations with and without disturbance are carried out and the results are analyzed. A battery test workbench is established and a Li-ion battery is applied to test the hardware in a loop experiment. Experimental results are plotted and analyzed according to the four aspects to evaluate the four model-based SOC estimation methods.

  13. Charge state distributions and charge-changing cross sections of heavy ions in the energy range up to 10 MeV/u

    International Nuclear Information System (INIS)

    Charge state distributions and charge-changing cross sections have been measured for heavy ions with atomic numbers between 18 and 92, in charge states from +9 to +68, and at energies in the range from 0.2 to 10 MeV/u using various gaseous and solid target materials. The experimental cross sections are compared with the theory of Bohr and Lindhard. The accuracy of predictions by means of known empirical formulae for average equilibrium charge states is briefly discussed. (author)

  14. State of Charge Estimation of Lithium-Ion Batteries Using an Adaptive Cubature Kalman Filter

    Directory of Open Access Journals (Sweden)

    Bizhong Xia

    2015-06-01

    Full Text Available Accurate state of charge (SOC estimation is of great significance for a lithium-ion battery to ensure its safe operation and to prevent it from over-charging or over-discharging. However, it is difficult to get an accurate value of SOC since it is an inner sate of a battery cell, which cannot be directly measured. This paper presents an Adaptive Cubature Kalman filter (ACKF-based SOC estimation algorithm for lithium-ion batteries in electric vehicles. Firstly, the lithium-ion battery is modeled using the second-order resistor-capacitor (RC equivalent circuit and parameters of the battery model are determined by the forgetting factor least-squares method. Then, the Adaptive Cubature Kalman filter for battery SOC estimation is introduced and the estimated process is presented. Finally, two typical driving cycles, including the Dynamic Stress Test (DST and New European Driving Cycle (NEDC are applied to evaluate the performance of the proposed method by comparing with the traditional extended Kalman filter (EKF and cubature Kalman filter (CKF algorithms. Experimental results show that the ACKF algorithm has better performance in terms of SOC estimation accuracy, convergence to different initial SOC errors and robustness against voltage measurement noise as compared with the traditional EKF and CKF algorithms.

  15. X-Ray Spectroscopy: An Experimental Technique to Measure Charge State Distribution Right at the Ion-Solid Interaction

    CERN Document Server

    Sharma, Prashant

    2015-01-01

    Charge state distributions of $^{56}$Fe and $^{58}$Ni projectile ions passing through thin carbon foils have been studied in the energy range of 1.44 - 2.69 MeV/u using a novel method from the x-ray spectroscopy technique. Interestingly the charge state distribution in the bulk show Lorentzian behavior instead of usual Gaussian distribution. Further, different parameters of charge state distribution like mean charge state, distribution width and asymmetric parameter are determined and compared with the empirical calculations and ETACHA predictions. It is found that the x-ray measurement technique is appropriate to determine the mean charge state right at the interaction zone or in the bulk. Interestingly, empirical formalism predicts much lower projectile mean charge states compare to x-ray measurements which clearly indicate multi-electron capture from the target surface. The ETACHA predictions and experimental results are found to be comparable for energies $\\geq$ 2 MeV/u.

  16. Energy loss of high velocity 6Li2+ ions in carbon foils in charge state non-equilibrium region

    International Nuclear Information System (INIS)

    Mean energy losses of high velocity H-like Li ions in thin carbon foils were measured in the charge state non-equilibrium region. Owing to the screening effect of the bound electron, the fixed-charge stopping power for 6Li2+ was smaller than that for 6Li3+. The projectile atomic number dependence of the fixed-charge stopping powers for H-like ions is discussed including our previous data of He, C and O ions with the same velocity. The present result is also compared with the theoretical prediction. (orig.)

  17. Extension of charge-state-distribution calculations for ion-solid collisions towards low velocities and many-electron ions

    Science.gov (United States)

    Lamour, E.; Fainstein, P. D.; Galassi, M.; Prigent, C.; Ramirez, C. A.; Rivarola, R. D.; Rozet, J.-P.; Trassinelli, M.; Vernhet, D.

    2015-10-01

    Knowledge of the detailed evolution of the whole charge-state distribution of projectile ions colliding with targets is required in several fields of research such as material science and atomic and nuclear physics but also in accelerator physics, and in particular in regard to the several foreseen large-scale facilities. However, there is a lack of data for collisions in the nonperturbative energy domain and that involve many-electron projectiles. Starting from the etacha model we developed [Rozet et al., Nucl. Instrum. Methods Phys. Res., Sect. B 107, 67 (1996), 10.1016/0168-583X(95)00800-4], we present an extension of its validity domain towards lower velocities and larger distortions. Moreover, the system of rate equations is able to take into account ions with up to 60 orbital states of electrons. The computed data from the different new versions of the etacha code are compared to some test collision systems. The improvements made are clearly illustrated by 28.9 MeV u-1P b56 + ions, and laser-generated carbon ion beams of 0.045 to 0.5 MeV u-1 , passing through carbon or aluminum targets, respectively. Hence, those new developments can efficiently sustain the experimental programs that are currently in progress on the "next-generation" accelerators or laser facilities.

  18. Projectile- and charge-state-dependent electron yields from ion penetration of solids as a probe of preequilibrium stopping power

    DEFF Research Database (Denmark)

    Rothard, H.; Schou, Jørgen; Groeneveld, K.-O.

    1992-01-01

    Kinetic electron-emission yields gamma from swift ion penetration of solids are proportional to the (electronic) stopping power gamma approximately Beta-S*, if the preequilibrium evolution of the charge and excitation states of the positively charged ions is taken into account. We show that the...... theory after having presented a summary of recent results on the projectile- and charge-state dependence of forward and backward electron yields gamma(F) and gamma(B) and the Meckbach factor R = gamma(F)/gamma(B). A simple extension of the yield equations is proposed and several assumptions are justified...

  19. The beam commissioning of a CW high charge state heavy ion RFQ

    Science.gov (United States)

    Zhu, K.; Lu, Y. R.; Yin, X. J.; Yang, Y. Q.; Gao, S. L.; Wang, Z.; He, Y.; Liu, G.; Zhang, X. H.; Yuan, Y. J.; Zhao, H. W.; Xia, J. W.; Chen, C. E.

    2015-09-01

    The SSC-LINAC project is launched at Institute of Modern Physics in China to develop one new linear accelerator (LINAC) injector for separated sector cyclotron (SSC). It includes a high charge state ion source, a CW RFQ and a DTL section, and is designed to accelerate ions up to 580 keV/u. Now the ion source and the RFQ cavity have been installed in the main hall and the beam commissioning has been carried out. Two kinds of ions have been tested, 16O5+ and 40Ar8+. The experiment result of 16O5+ is: the measured beam current is 180 μA at entrance of RFQ and 150 μA at exit of RFQ. The output energy of 16O5+ is 141.89 keV/u. The measured beam current is 210 μA at entrance of RFQ and 198 μA at exit of RFQ for 40Ar8+. The output energy of 40Ar8+ is 142.78 keV/u. The experiment results agree with the design parameters of RFQ very well. This paper presents: the design consideration of beam dynamics, RF and cooling structure design; measurement of the cold model; high power test of RFQ and beam commissioning result.

  20. The beam commissioning of a CW high charge state heavy ion RFQ

    International Nuclear Information System (INIS)

    The SSC-LINAC project is launched at Institute of Modern Physics in China to develop one new linear accelerator (LINAC) injector for separated sector cyclotron (SSC). It includes a high charge state ion source, a CW RFQ and a DTL section, and is designed to accelerate ions up to 580 keV/u. Now the ion source and the RFQ cavity have been installed in the main hall and the beam commissioning has been carried out. Two kinds of ions have been tested, 16O5+ and 40Ar8+. The experiment result of 16O5+ is: the measured beam current is 180 μA at entrance of RFQ and 150 μA at exit of RFQ. The output energy of 16O5+ is 141.89 keV/u. The measured beam current is 210 μA at entrance of RFQ and 198 μA at exit of RFQ for 40Ar8+. The output energy of 40Ar8+ is 142.78 keV/u. The experiment results agree with the design parameters of RFQ very well. This paper presents: the design consideration of beam dynamics, RF and cooling structure design; measurement of the cold model; high power test of RFQ and beam commissioning result

  1. Bound state properties and photo-detachment of the negatively charged hydrogen ions

    International Nuclear Information System (INIS)

    The absorption of infrared and visible radiation from stellar emission spectra by the negatively charged hydrogen ions H- is considered. The explicit formula for the photo-detachment cross-section of the negatively charged hydrogen ion(s) is derived. Photo-detachment cross-sections of the ∞H-, 3H- (or T-), 2H- (or D-) and 1H- ions are determined to high accuracy and for a large number of photo-electron momenta/energies. We introduce criteria which can be used to evaluate the overall quality of highly accurate wave functions of the hydrogen ion(s). One of these criteria is based on highly accurate calculations of the lowest order QED corrections in the negatively charged hydrogen ions, including 1H- (protium), 2H- (deuterium), 3H- (tritium) and model ion with the infinitely heavy nucleus ∞H-. An effective approach has been developed to calculate three-body integrals with the Bessel functions of different orders. Some preliminary evaluations of the photo-detachment cross-sections of the negatively charged hydrogen ions are performed. Inverse Bremsstrahlung in the field of the neutral hydrogen atom is briefly discussed. (author)

  2. Ionization and bound-state relativistic quantum dynamics in laser-driven multiply charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Hetzheim, Henrik

    2009-01-14

    The interaction of ultra-strong laser fields with multiply charged hydrogen-like ions can be distinguished in an ionization and a bound dynamics regime. Both are investigated by means of numerically solving the Dirac equation in two dimensions and by a classical relativistic Monte-Carlo simulation. For a better understanding of highly nonlinear physical processes the development of a well characterized ultra-intense relativistic laser field strength has been driven forward, capable of studying e.g. the magnetic field effects of the laser resulting in an additional electron motion in the laser propagation direction. A novel method to sensitively measure these ultra-strong laser intensities is developed and employed from the optical via the UV towards the XUV frequency regime. In the bound dynamics field, the determination of multiphoton transition matrixelements has been investigated between different bound states via Rabi oscillations. (orig.)

  3. Ionization and bound-state relativistic quantum dynamics in laser-driven multiply charged ions

    International Nuclear Information System (INIS)

    The interaction of ultra-strong laser fields with multiply charged hydrogen-like ions can be distinguished in an ionization and a bound dynamics regime. Both are investigated by means of numerically solving the Dirac equation in two dimensions and by a classical relativistic Monte-Carlo simulation. For a better understanding of highly nonlinear physical processes the development of a well characterized ultra-intense relativistic laser field strength has been driven forward, capable of studying e.g. the magnetic field effects of the laser resulting in an additional electron motion in the laser propagation direction. A novel method to sensitively measure these ultra-strong laser intensities is developed and employed from the optical via the UV towards the XUV frequency regime. In the bound dynamics field, the determination of multiphoton transition matrixelements has been investigated between different bound states via Rabi oscillations. (orig.)

  4. Adaptive unscented Kalman filtering for state of charge estimation of a lithium-ion battery for electric vehicles

    International Nuclear Information System (INIS)

    An accurate battery State of Charge estimation is of great significance for battery electric vehicles and hybrid electric vehicles. This paper presents an adaptive unscented Kalman filtering method to estimate State of Charge of a lithium-ion battery for battery electric vehicles. The adaptive adjustment of the noise covariances in the State of Charge estimation process is implemented by an idea of covariance matching in the unscented Kalman filter context. Experimental results indicate that the adaptive unscented Kalman filter-based algorithm has a good performance in estimating the battery State of Charge. A comparison with the adaptive extended Kalman filter, extended Kalman filter, and unscented Kalman filter-based algorithms shows that the proposed State of Charge estimation method has a better accuracy. -- Highlights: → Adaptive unscented Kalman filtering is proposed to estimate State of Charge of a lithium-ion battery for electric vehicles. → The proposed method has a good performance in estimating the battery State of Charge. → A comparison with three other Kalman filtering algorithms shows that the proposed method has a better accuracy.

  5. Gas-pressure dependence of charge-state fractions and mean charges of 1.4 MeV/u-uranium ions stripped in molecular hydrogen

    Science.gov (United States)

    Shevelko, V. P.; Winckler, N.; Tolstikhina, I. Yu.

    2016-06-01

    Using a recently created BREIT computer code (Balance Rate Equations for Ion Transportation), evolutions of the charge-state fractions Fq (x) and equilibrium mean charge states q bar are calculated for stripping of 1.4 MeV/u-U4+ ions in H2 gas for target thicknesses x ⩽ 100 μg /cm2 (⩽ 3 ·1019molecule /cm2) and gas pressures 10-4 ⩽ P ⩽ 500 mbar. Calculations of the non-equilibrium Fq (x) and equilibrium Fq0 distributions for ion charges 4 ⩽ q ⩽ 40 are performed by solving the balance (rate) equations with account for the multi-electron processes and the target-density effect. Calculated equilibrium mean charge state increases from q bar ≈ 27.6 at P =10-4 mbar to its saturated (maximum) value of q bar ≈ 32.7 at pressures P≳ 250 mbar while the equilibrium target thickness xeq increases from 20 to 50 μg /cm2 (from 0.6 to 1.5 in units of 1019molecule /cm2) in the H2-pressure range considered. From the present calculations it is concluded that the maximum mean charge state q bar which can be achieved in stripping of 1.4 MeV/u-U4+ ions in H2 gas is about q bar ≈ 33 at a gas pressure P≳ 250 mbar.

  6. Calculations on charge state and energy loss of argon ions in partially and fully ionized carbon plasmas.

    Science.gov (United States)

    Barriga-Carrasco, Manuel D; Casas, David; Morales, Roberto

    2016-03-01

    The energy loss of argon ions in a target depends on their velocity and charge density. At the energies studied in this work, it depends mostly on the free and bound electrons in the target. Here the random-phase approximation is used for analyzing free electrons at any degeneracy. For the plasma-bound electrons, an interpolation between approximations for low and high energies is applied. The Brandt-Kitagawa (BK) model is employed to depict the projectile charge space distribution, and the stripping criterion of Kreussler et al. is used to determine its equilibrium charge state Q(eq). This latter criterion implies that the equilibrium charge state depends slightly on the electron density and temperature of the plasma. On the other hand, the effective charge Q(eff) is obtained as the ratio between the energy loss of the argon ion and that of the proton for the same plasma conditions. This effective charge Q(eff) is larger than the equilibrium charge state Q(eq) due to the incorporation of the BK charge distribution. Though our charge-state estimations are not exactly the same as the experimental values, our energy loss agrees quite well with the experiments. It is noticed that the energy loss in plasmas is higher than that in the same cold target of about, ∼42-62.5% and increases with carbon plasma ionization. This confirms the well-known enhanced plasma stopping. It is also observed that only a small part of this energy loss enhancement is due to an increase of the argon charge state, namely only ∼2.2 and 5.1%, for the partially and the fully ionized plasma, respectively. The other contribution is connected with a better energy transfer to the free electrons at plasma state than to the bound electrons at solid state of about, ∼38.8-57.4%, where higher values correspond to a fully ionized carbon plasma. PMID:27078472

  7. Calculations on charge state and energy loss of argon ions in partially and fully ionized carbon plasmas

    Science.gov (United States)

    Barriga-Carrasco, Manuel D.; Casas, David; Morales, Roberto

    2016-03-01

    The energy loss of argon ions in a target depends on their velocity and charge density. At the energies studied in this work, it depends mostly on the free and bound electrons in the target. Here the random-phase approximation is used for analyzing free electrons at any degeneracy. For the plasma-bound electrons, an interpolation between approximations for low and high energies is applied. The Brandt-Kitagawa (BK) model is employed to depict the projectile charge space distribution, and the stripping criterion of Kreussler et al. is used to determine its equilibrium charge state Qeq. This latter criterion implies that the equilibrium charge state depends slightly on the electron density and temperature of the plasma. On the other hand, the effective charge Qeff is obtained as the ratio between the energy loss of the argon ion and that of the proton for the same plasma conditions. This effective charge Qeff is larger than the equilibrium charge state Qeq due to the incorporation of the BK charge distribution. Though our charge-state estimations are not exactly the same as the experimental values, our energy loss agrees quite well with the experiments. It is noticed that the energy loss in plasmas is higher than that in the same cold target of about, ˜42 -62.5 % and increases with carbon plasma ionization. This confirms the well-known enhanced plasma stopping. It is also observed that only a small part of this energy loss enhancement is due to an increase of the argon charge state, namely only ˜2.2 and 5.1 % , for the partially and the fully ionized plasma, respectively. The other contribution is connected with a better energy transfer to the free electrons at plasma state than to the bound electrons at solid state of about, ˜38.8 -57.4 % , where higher values correspond to a fully ionized carbon plasma.

  8. Aerosol charging state at an urban site: new analytical approach and implications for ion-induced nucleation

    Directory of Open Access Journals (Sweden)

    S. Gagné

    2012-05-01

    Full Text Available The charging state of aerosol populations was determined using an Ion-DMPS in Helsinki, Finland between December 2008 and February 2010. We extrapolated the charging state and calculated the ion-induced nucleation fraction to be around 1.3 % ± 0.4 % at 2 nm and 1.3 % ± 0.5 % at 1.5 nm, on average. We present a new method to retrieve the average charging state for a new particle formation event, at a given size and polarity. We improve the uncertainty assessment and fitting technique used previously with an Ion-DMPS. We also use a new theoretical framework that allows for different concentrations of small ions for different polarities (polarity asymmetry. We extrapolate the ion-induced fraction using polarity symmetry and asymmetry. Finally, a method to calculate the growth rates from the behaviour of the charging state as a function of the particle diameter using polarity symmetry and asymmetry is presented and used on a selection of new particle formation events.

  9. Recent developments in high charge state heavy ion beams at the LBL 88-inch cyclotron

    International Nuclear Information System (INIS)

    Recent advances in design and operation of the internal PIG sources at the LBL 88-Inch Cyclotron have led to the development of high charge state (0.4 less than or equal to Q/A less than or equal to 0.5) heavy ion beams between lithium and neon with energies 20 less than or equal to E/A/ less than or equal to 32 MeV per nucleon, including fully stripped ions up to 16O8+. Total external intensities of these beams range from 1012 particles/s for 6Li3+ to 0.1 particles/s for 16O8+. Techniques have been developed for routine tune-out of the low intensity beams. These include use of model beams and reliance on the large systematic data base of cyclotron parameters which has been developed over many years of operation. Techniques for delivery of these weak beams to the experimental target areas are presented. Source design and operation, including special problems associated with Li, Be and B beams, are discussed

  10. Charge state evolution in an ion trap irradiated by VUV synchrotron radiation

    International Nuclear Information System (INIS)

    The energies of photons obtainable from the VUV ring at the National Synchrotron Light Source (NSLS) are ideally suited for high-efficiency ionization of atomic outer-shell electrons. Given the high fluxes of photons available on a wiggler beam line, multiple photoionization in an ion trap can be easily achieved within times short compared to typical ion storage times in the trap. Measurements of the time evolution of ion populations in such a trap can yield ionic photoionization cross sections and charge-exchange interaction rates for ion-atom or ion-ion collisions. The various processes governing this time evolution are discussed and model calculations illustrating the relative importance of these processes under different conditions are presented. 8 refs., 5 figs., 1 tab

  11. Combined State of Charge and State of Health estimation over lithium-ion battery cell cycle lifespan for electric vehicles

    Science.gov (United States)

    Zou, Yuan; Hu, Xiaosong; Ma, Hongmin; Li, Shengbo Eben

    2015-01-01

    A combined SOC (State Of Charge) and SOH (State Of Health) estimation method over the lifespan of a lithium-ion battery is proposed. First, the SOC dependency of the nominal parameters of a first-order RC (resistor-capacitor) model is determined, and the performance degradation of the nominal model over the battery lifetime is quantified. Second, two Extended Kalman Filters with different time scales are used for combined SOC/SOH monitoring: the SOC is estimated in real-time, and the SOH (the capacity and internal ohmic resistance) is updated offline. The time scale of the SOH estimator is determined based on model accuracy deterioration. The SOC and SOH estimation results are demonstrated by using large amounts of testing data over the battery lifetime.

  12. State-Selective Quantum Interference Observed in the Recombination of Highly Charged Hg75+···78+ Mercury Ions in an Electron Beam Ion Trap

    International Nuclear Information System (INIS)

    We present experimental data on the state-selective quantum interference between different pathways of photorecombination, namely, radiative and dielectronic recombination, in the KLL resonances of highly charged mercury ions. The interference, observed for well resolved electronic states in the Heidelberg electron beam ion trap, manifests itself in the asymmetry of line shapes, characterized by ''Fano factors,'' which have been determined with unprecedented precision, as well as their excitation energies, for several strong dielectronic resonances

  13. Experimental study of ion stopping power in warm dense matter: charge-state distribution measurements of ions leaving warm dense matter

    International Nuclear Information System (INIS)

    The determination if the ion slowing down process (or stopping power) in warm dense matter is essential especially in the frame of inertial confinement fusion. During my thesis, our interest was driven by the modification of the charge state of ion beam emerging from warm dense matter, this quantity playing a major role in ion stopping power calculation. We took advantage of the properties exhibited by ion beams produced by high intensity short pulse lasers to study during two experiments performed at ELFIE and TITAN facilities, the charge state modification of a carbon and helium ion beams emerging from an aluminum foil isochorically heated by an energetic proton beam. In the first two chapters are presented the major challenges regarding the subject from both a theoretical and experimental point of view. Here are exposed the different simulation tools used during the thesis. The third chapter is devoted to the study of the property of laser-produced ion beams in the scope of our experiments aiming at studying the stopping power. We have studied in particular ion beams generated using lower-than-solid density targets during two experiments: helium gas jet and laser-exploded target. In the last chapter are presented the set-ups and results of the two experiments on the charge state of ion beam emerging from warm dense matter. The data we measured in solid-density cold aluminum are successfully compared with the results already obtained in conventional accelerators. (author)

  14. State-diagnosed charge stripping in low-energy collisions of ground-state and highly excited N+ ions with He

    International Nuclear Information System (INIS)

    Translational energy spectra have been measured on N2+ product ions resulting from 2-keV charge-stripping collisions between N+ ions and He. The projectile N+ ion beam is produced under varying ion source conditions so as to contain different fractions of a long-lived metastable component. By measuring the endoergic energy defect for charge stripping from ground-state and excited-state projectiles at different electron energies in the ion source, the quantal identity of the N+ metastable state is deduced to be either 2s2p22p' 1D0, which lies 17.9 eV above the 2s22p23P ground electronic state, or 2s22p3s 1P0, whose excitation energy is 18.5 eV

  15. Dynamics of the Rydberg state population of slow highly charged ions impinging a solid surface at arbitrary collision geometry

    Science.gov (United States)

    Nedeljković, N. N.; Majkić, M. D.; Božanić, D. K.; Dojčilović, R. J.

    2016-06-01

    We consider the population dynamics of the intermediate Rydberg states of highly charged ions (core charge Z\\gg 1, principal quantum number {n}{{A}}\\gg 1) interacting with solid surfaces at arbitrary collision geometry. The recently developed resonant two-state vector model for the grazing incidence (2012 J. Phys. B: At. Mol. Opt. Phys. 45 215202) is extended to the quasi-resonant case and arbitrary angle of incidence. According to the model, the population probabilities depend both on the projectile parallel and perpendicular velocity components, in a complementary way. A cascade neutralization process for {{{Xe}}}Z+ ions, for Z=15{--}45, interacting with a conductive-surface is considered by taking into account the population dynamics. For an arbitrary collision geometry and given range of ionic velocities, a micro-staircase model for the simultaneous calculation of the kinetic energy gain and the charge state of the ion in front of the surface is proposed. The relevance of the obtained results for the explanation of the formation of nanostructures on solid surfaces by slow highly charged ions for normal incidence geometry is briefly discussed.

  16. State of Charge Dependent Mechanical Integrity Behavior of 18650 Lithium-ion Batteries.

    Science.gov (United States)

    Xu, Jun; Liu, Binghe; Hu, Dayong

    2016-01-01

    Understanding the mechanism of mechanical deformation/stress-induced electrical failure of lithium-ion batteries (LIBs) is important in crash-safety design of power LIBs. The state of charge (SOC) of LIBs is a critical factor in their electrochemical performance; however, the influence of SOC with mechanical integrity of LIBs remains unclear. This study investigates the electrochemical failure behaviors of LIBs with various SOCs under both compression and bending loadings, underpinned by the short circuit phenomenon. Mechanical behaviors of the whole LIB body, which is regarded as an intact structure, were analyzed in terms of structure stiffness. Results showed that the mechanical behaviors of LIBs depend highly on SOC. Experimental verification on the cathode and anode sheet compression tests show that higher SOC with more lithium inserted in the anode leads to higher structure stiffness. In the bending tests, failure strain upon occurrence of short circuit has an inverse linear relationship with the SOC value. These results may shed light on the fundamental physical mechanism of mechanical integrity LIBs in relation to inherent electrochemical status. PMID:26911922

  17. Quightness: A proposed figure of merit for sources of low-energy, high-charge-state ions

    International Nuclear Information System (INIS)

    A variety of ion sources, including the EBIS and ECRIS, are distinguished by their ability to produce low-energy ions of very high charge state. It would be useful to have some figure of merit that is particularly sensitive to this performance. I propose here such a quantity, called ''Quightness,'' which is related to brightness but which enhances the contrast between sources supplying multicharged ions of low energy. The rationale for introducing this quantity, its etymology and relationship to other figures of merit, and some representative values are presented

  18. Spatially resolved charge-state and current-density distributions at the extraction of an electron cyclotron resonance ion source

    International Nuclear Information System (INIS)

    In this paper we present our measurements of charge-state and current-density distributions performed in very close vicinity (15 mm) of the extraction of our hexapole geometry electron cyclotron resonance ion source. We achieved a relatively high spatial resolution reducing the aperture of our 3D-movable extraction (puller) electrode to a diameter of only 0.5 mm. Thus, we are able to limit the source of the extracted ion beam to a very small region of the plasma electrode's hole (O = 4 mm) and therefore to a very small region of the neutral plasma sheath. The information about the charge-state distribution and the current density in the plane of the plasma electrode at each particular position is conserved in the ion beam. We determined the total current density distribution at a fixed coaxial distance of only 15 mm to the plasma electrode by remotely moving the small-aperture puller electrode which contained a dedicated Faraday cup (FC) across the aperture of the plasma electrode. In a second measurement we removed the FC and recorded m/q-spectra for the different positions using a sector magnet. From our results we can deduce that different ion charge-states can be grouped into bloated triangles of different sizes and same orientation at the extraction with the current density peaking at centre. This confirms observations from other groups based on simulations and emittance measurements. We present our measurements in detail and discuss possible systematic errors.

  19. Laser sources of multiply charged heavy ions

    International Nuclear Information System (INIS)

    Laser production of highly charged ions is studied at the 50 J photodissociation iodine laser facility PERUN. The laser beam is focused onto various metallic targets. The use of a parabolic mirror with a hole in the center instead of a focusing lens allows for measuring ion beam parameters along the laser beam axis and results in two fold increase in the ion extraction. The diagnostics of the laser-produced ions in a far expansion zone is based on the time-of-flight method. The reported results prove the existence of highly charged ions with ion charge z > 40 in a far expansion zone and their survival during the recombination processes occurring in early stages of expansion. The higher laser power density is applied the higher ion charge states are generated. The maximum ion charge achieved e.g. for tantalum was z = 55. (J.U.)

  20. Mean charge states of MeV/u Fe, Co, Ni and Cu ions in Au and Bi solid targets

    International Nuclear Information System (INIS)

    The average charge states of 0.1 - 1.5 MeV/u Fe, Co, Ni, and Cu ions in solid Au and Bi targets have been determined by estimating the mean numbers of outer-shell spectator vacancies during the K-vacancy decay. The latter quantities were obtained from the yield and energy shifts of the Kα,β X-rays, by comparing with calculations in the independent electron approximation. The reported equilibrium charges, mostly characteristic for the inside of the target, are in fairly agreement with Nikolaev and Dmitriev semi-empirical formula. (authors)

  1. Estimation of State of Charge of a Lithium-Ion Battery Pack for Electric Vehicles Using an Adaptive Luenberger Observer

    OpenAIRE

    Yuan Zou; Fengchun Sun; Xiaosong Hu

    2010-01-01

    In order to safely and efficiently use the power as well as to extend the lifetime of the traction battery pack, accurate estimation of State of Charge (SoC) is very important and necessary. This paper presents an adaptive observer-based technique for estimating SoC of a lithium-ion battery pack used in an electric vehicle (EV). The RC equivalent circuit model in ADVISOR is applied to simulate the lithium-ion battery pack. The parameters of the battery model as a function of SoC, are identifi...

  2. Cross-sections for electron capture by multiply charged ions from hydrogen atoms and molecules and population of electronic states of created ions

    International Nuclear Information System (INIS)

    The cross-sections for single electron capture by alpha-particles and multiply charged ions Ne3+, Ne4+, Ar4+, Ar5+, Ar6+ from hydrogen atoms and molecules have been measured using registration of coincidences between incident and recoil ions after collision to separate this process. Population of different electronic states of ions with lower charges produced at single electron capture has been measured by collision spectroscopy method. Cross-sections for one electron capture by He2+, ArZ+ (Z = 6, 5, 4) and NeZ+ (Z = 3-4) have been measured in the kinetic energy range of incident multiply charged ions from 1xZ to 12xZ keV (Z is charge of multiply charged ions). Cross-sections for the population of electronic states at electron capture from H2 molecules have been measured in the velocity range from V = 1·107 cm/s to V5,5·107 cm/s (in the collision energy range 3.0xZ Kev - 21.0xZ KeV) at collisions of ArZ+ ions (Z=3-6) and NeZ+ (Z3-4). The double electron capture cross-sections at incident alpha-particles and hydrogen molecules collision have been measured in the energy range from 1 KeV up to 100 KeV (V=0, 235/2, 58·108 cm/s). Errors of measured values of cross-sections are ∼10-15% The results of the measurements are presented in Tables 1-8. (author)

  3. On-line parameter, state-of-charge and aging estimation of Li-ion batteries

    NARCIS (Netherlands)

    Rosca, B.; Kessels, J.T.B.A.; Bergveld, H.J.; Bosch, P.P.J. van den

    2012-01-01

    This paper presents an on-line model identification method for Li-ion battery parameters that combines high accuracy and low computational complexity. Experimental results show that modeling errors are smaller than 1% throughout the feasible operating range. The identified model is used in a state o

  4. Generation of high charge state metal ion beams by electron cyclotron resonance heating of vacuum arc plasma in cusp trap.

    Science.gov (United States)

    Nikolaev, A G; Savkin, K P; Oks, E M; Vizir, A V; Yushkov, G Yu; Vodopyanov, A V; Izotov, I V; Mansfeld, D A

    2012-02-01

    A method for generating high charge state heavy metal ion beams based on high power microwave heating of vacuum arc plasma confined in a magnetic trap under electron cyclotron resonance conditions has been developed. A feature of the work described here is the use of a cusp magnetic field with inherent "minimum-B" structure as the confinement geometry, as opposed to a simple mirror device as we have reported on previously. The cusp configuration has been successfully used for microwave heating of gas discharge plasma and extraction from the plasma of highly charged, high current, gaseous ion beams. Now we use the trap for heavy metal ion beam generation. Two different approaches were used for injecting the vacuum arc metal plasma into the trap--axial injection from a miniature arc source located on-axis near the microwave window, and radial injection from sources mounted radially at the midplane of the trap. Here, we describe preliminary results of heating vacuum arc plasma in a cusp magnetic trap by pulsed (400 μs) high power (up to 100 kW) microwave radiation at 37.5 GHz for the generation of highly charged heavy metal ion beams. PMID:22380156

  5. Negative-continuum dielectronic recombination into excited states of highly-charged ions

    OpenAIRE

    Artemyev, A. N.; Shabaev, V. M.; Stöhlker, Th; Surzhykov, A. S.

    2009-01-01

    The recombination of a free electron into a bound state of bare, heavy nucleus under simultaneous production of bound-electron--free-positron pair is studied within the framework of relativistic first--order perturbation theory. This process, denoted as "negative-continuum dielectronic recombination" leads to a formation of not only the ground but also the singly- and doubly-excited states of the residual helium-like ion. The contributions from such an excited--state capture to the total as w...

  6. Excited State Formation in Electron Capture by Slow Multiply Charged Ions

    International Nuclear Information System (INIS)

    Translational energy spectroscopy (TES) has been used to study one-electron capture by H and He-like ions of C, N and O in both H and H2 at energies below 1 keV amu-1. Similar measurements have been carried out for He2+ ions in the hydrocarbons CH4, C2H4, C2H6 and H2O at energies within the range 250-2000 eV amu-1. One-electron capture by O6+ ions in H2O, CO2 and CH4 and by C4+ ions in CH4 have also been studied in the range 200-1500 eV amu-1. The main excited product states have been identified, their relative importance assessed and, in some cases, cross-sections determined. In the molecular targets, contributions to one-electron capture from non-dissociative and dissociative mechanisms as well as from two-electron capture into autoionizing states has also been determined. In all cases, the highly selective nature of the electron capture process is confirmed even in the case of molecules with many possible fragmentation channels involving a wide range of energy defects. In the case of H, the main product channels are well predicted by reaction windows calculated using a Landau-Zener approach. However, the same approach applied to molecules, where both non-dissociative and dissociative mechanisms are significant, is found to be of limited use. (author)

  7. EVOLUTION OF THE RELATIONSHIPS BETWEEN HELIUM ABUNDANCE, MINOR ION CHARGE STATE, AND SOLAR WIND SPEED OVER THE SOLAR CYCLE

    International Nuclear Information System (INIS)

    The changing relationships between solar wind speed, helium abundance, and minor ion charge state are examined over solar cycle 23. Observations of the abundance of helium relative to hydrogen (AHe ≡ 100 × nHe/nH) by the Wind spacecraft are used to examine the dependence of AHe on solar wind speed and solar activity between 1994 and 2010. This work updates an earlier study of AHe from 1994 to 2004 to include the recent extreme solar minimum and broadly confirms our previous result that AHe in slow wind is strongly correlated with sunspot number, reaching its lowest values in each solar minima. During the last minimum, as sunspot numbers reached their lowest levels in recent history, AHe continued to decrease, falling to half the levels observed in slow wind during the previous minimum and, for the first time observed, decreasing even in the fastest solar wind. We have also extended our previous analysis by adding measurements of the mean carbon and oxygen charge states observed with the Advanced Composition Explorer spacecraft since 1998. We find that as solar activity decreased, the mean charge states of oxygen and carbon for solar wind of a given speed also fell, implying that the wind was formed in cooler regions in the corona during the recent solar minimum. The physical processes in the coronal responsible for establishing the mean charge state and speed of the solar wind have evolved with solar activity and time.

  8. State-Of-Charge Estimation of Li-Ion Battery Using Extended Kalman Filter

    OpenAIRE

    Feng Jin; He Yong-ling

    2013-01-01

    The Li-ion battery is studied base on its equivalent circuit PNGV model. The model parameters are identified by HPPC test. The discrete state space equation is established according to the model. The basic theory of extended Kalman filter algorithm is studied and then the filtering algorithm is set up under the noisy environments. Finally, a kind of electric car is used for testing under the UDDS driving condition. The difference between the simulation value using extended Kalman filter under...

  9. Estimation of State of Charge for Two Types of Lithium-Ion Batteries by Nonlinear Predictive Filter for Electric Vehicles

    Directory of Open Access Journals (Sweden)

    Yin Hua

    2015-04-01

    Full Text Available Estimation of state of charge (SOC is of great importance for lithium-ion (Li-ion batteries used in electric vehicles. This paper presents a state of charge estimation method using nonlinear predictive filter (NPF and evaluates the proposed method on the lithium-ion batteries with different chemistries. Contrary to most conventional filters which usually assume a zero mean white Gaussian process noise, the advantage of NPF is that the process noise in NPF is treated as an unknown model error and determined as a part of the solution without any prior assumption, and it can take any statistical distribution form, which improves the estimation accuracy. In consideration of the model accuracy and computational complexity, a first-order equivalent circuit model is applied to characterize the battery behavior. The experimental test is conducted on the LiCoO2 and LiFePO4 battery cells to validate the proposed method. The results show that the NPF method is able to accurately estimate the battery SOC and has good robust performance to the different initial states for both cells. Furthermore, the comparison study between NPF and well-established extended Kalman filter for battery SOC estimation indicates that the proposed NPF method has better estimation accuracy and converges faster.

  10. HICS: Highly charged ion collisions with surfaces

    OpenAIRE

    Peters, Thorsten; Haake, Christian; Hopster, Johannes; Sokolovsky, Valentin; Wucher, Andreas; Schleberger, Marika

    2008-01-01

    The layout of a new instrument designed to study the interaction of highly charged ions with surfaces, which consists of an ion source, a beamline including charge separation and a target chamber, is presented here. By varying the charge state and impact velocity of the projectiles separately, the dissipation of potential and kinetic energy at or below the surface can be studied independently. The target chamber offers the use of tunable metal-insulator-metal devices as detectors for internal...

  11. State of charge modeling of lithium-ion batteries using dual exponential functions

    Science.gov (United States)

    Kuo, Ting-Jung; Lee, Kung-Yen; Huang, Chien-Kang; Chen, Jau-Horng; Chiu, Wei-Li; Huang, Chih-Fang; Wu, Shuen-De

    2016-05-01

    A mathematical model is developed by fitting the discharging curve of LiFePO4 batteries and used to investigate the relationship between the state of charge and the closed-circuit voltage. The proposed mathematical model consists of dual exponential terms and a constant term which can fit the characteristics of dual equivalent RC circuits closely, representing a LiFePO4 battery. One exponential term presents the stable discharging behavior and the other one presents the unstable discharging behavior and the constant term presents the cut-off voltage.

  12. Equilibrium and non-equilibrium charge-state distributions of 2.0 MeV/u carbon ions passing through carbon foils

    International Nuclear Information System (INIS)

    Both equilibrium and non-equilibrium charge-state distributions were studied experimentally for 2.0 MeV/u carbon ions after passing through carbon foils. Measured charge-state distribution established the equilibrium at a target thickness of 10 μg/cm2 and this remained unchanged until a maximum target thickness of 98 μg/cm2. The equilibrium charge-state distribution, the equilibrium mean charge-state, and the width and skewness of the equilibrium distribution were compared with predictions using existing semi-empirical formulae as well as simulation results, including the ETACHA code. It was found that charge-state distributions, mean charge states, and distribution widths for C2+, C3+, and C4+ incident ions merged into quasi-equilibrium values at a target thickness of 5.7 μg/cm2 in the pre-equilibrium region and evolved simultaneously to the ‘real equilibrium’ values for all of the initial charge states, including C5+ and C6+ ions, as previously demonstrated for sulfur projectile ions at the same velocity (Imai et al., 2009). Two kinds of simulation, ETACHA and solution of rate equations taking only single electron transfers into account, were used, and both of them reproduced the measured charge evolution qualitatively. The quasi-equilibrium behavior could be reproduced with the ETACHA code, but not with solution of elementary rate equations

  13. Production and physics of highly charged ions

    International Nuclear Information System (INIS)

    Highly charged ions with very few electrons make a novel and attractive research object in atomic physics. High precision spectroscopy of such ions provides a powerful tool for exploring relativistic and quantum electrodynamic effects. Moreover, their enormous electro static potential gives rise to conspicuous effects during their interaction with other particles or matters. Study of the highly charged ions may thus open up a hitherto unexplored realm of physics, shedding light on giant resonance due to multi-hole states, multiply-excited resonances displaying strong electron correlations, etc. While this comprehensive study of highly charged ions is aimed at contributing to fundamental science, spinoff should contribute to such areas as the X-ray laser, nuclear fusion and space science. In spite of their importance, it is not easy to produce these ions. Various laboratory sources are being developed. Among these, the Electron Beam Ion Source (EBIS) and the Electron Cyclotron Beam Ion Source (ECRIS) are the powerful ones and have the potential to produce ions of higher charge state, keeping the ion energy low. Our purpose here is both to summarize briefly the current state of the development for highly charged ion source, and to introduce a part of atomic physics experiments with the source. (author)

  14. Production of highly charged ion beams from ECR ion sources

    International Nuclear Information System (INIS)

    Electron Cyclotron Resonance (ECR) ion source development has progressed with multiple-frequency plasma heating, higher mirror magnetic fields and better technique to provide extra cold electrons. Such techniques greatly enhance the production of highly charged ions from ECR ion sources. So far at cw mode operation, up to 300 eμA of O7+ and 1.15 emA of O6+, more than 100 eμA of intermediate heavy ions for charge states up to Ar13+, Ca13+, Fe13+, Co14+ and Kr18+, and tens of eμA of heavy ions with charge states to Kr26+, Xe28+, Au35+, Bi34+ and U34+ have been produced from ECR ion sources. At an intensity of at least 1 eμA, the maximum charge state available for the heavy ions are Xe36+, Au46+, Bi47+ and U48+. An order of magnitude enhancement for fully stripped argon ions (I ≥ 60 enA) also has been achieved. This article will review the ECR ion source progress and discuss key requirement for ECR ion sources to produce the highly charged ion beams

  15. Ion charge state distributions in ECR-plasmas determined from mass spectrometry and X-ray spectroscopy

    International Nuclear Information System (INIS)

    The influence of microwave power, magnetic field, neutral gas pressure and gas mixture on the ion charge state distribution (CSD) of an electron cyclotron resonance (ECR) plasma was investigated by q/A-analysis of an ion beam extracted from the plasma and by X-ray spectroscopy of this plasma. As the ion beam expands from a limited plasma edge and the extraction process alters the plasma properties in this region a small plasma cone including the discharge core is investigated by the X-ray method. For this reason the measured CSD are significantly different. Additionally, the transmission of the ions to the beam stop depends on the q/A ratio of the ion species and can falsify the true, primary CSD. In this way, the analysis of ECR plasma X-rays represents a more accurate method to measure the CSD of a discharge. In comparison to the q/A analysis it provides the true distribution and, moreover, different plasma regions can be examined

  16. Scaling for state-selective charge exchange due to collisions of multicharged ions with hydrogen

    Science.gov (United States)

    Jorge, A.; Illescas, Clara; Miraglia, J. E.; Gravielle, M. S.

    2015-12-01

    In this article we evaluate state-resolved charge exchange cross sections for Be{}4+, {{{B}}}5+, {{{C}}}6+, {{{N}}}7+, and {{{O}}}8+ projectiles colliding with atomic hydrogen employing two different methods: the classical trajectory Monte Carlo and the eikonal impulse approximations. These cross sections are used to extend previously derived scaling laws for n-, nl-, and nlm-distributions to highly excited final levels with 4≤slant n≤slant 9, covering energies in the range 50-2000 {{keV}}/ amu. Present total and partial capture cross sections are in agreement with available experimental and theoretical data for these collision systems. Besides, the proposed scaling rules are also verified by other theories, becoming a useful instrument for plasma research.

  17. Beta decay of highly charged ions

    International Nuclear Information System (INIS)

    Ion storage rings and ion traps provide the very first opportunity to address nuclear beta decay under conditions prevailing in hot stellar plasmas during nucleosynthesis, i.e. at high atomic charge states. Experiments are summarized that were performed in this field during the last decade at the ion storage-cooler ring ESR in Darmstadt. Special emphasis is given to the first observation of bound-state beta decay, where the created electron remains bound in an inner orbital of the daughter atom. The impact of this specific 'stellar' decay mode for s-process nucleosynthesis as well as for nuclear 'eon clocks' is outlined. Finally, a new technique, single-ion decay spectroscopy, is presented, where one observes two-body beta decay characteristics (i.e. orbital electron capture or bound-state beta decay) of highly charged, single ions for well-defined nuclear and atomic quantum states of both the mother - and the daughter - ion.

  18. Estimation of State of Charge of a Lithium-Ion Battery Pack for Electric Vehicles Using an Adaptive Luenberger Observer

    Directory of Open Access Journals (Sweden)

    Yuan Zou

    2010-09-01

    Full Text Available In order to safely and efficiently use the power as well as to extend the lifetime of the traction battery pack, accurate estimation of State of Charge (SoC is very important and necessary. This paper presents an adaptive observer-based technique for estimating SoC of a lithium-ion battery pack used in an electric vehicle (EV. The RC equivalent circuit model in ADVISOR is applied to simulate the lithium-ion battery pack. The parameters of the battery model as a function of SoC, are identified and optimized using the numerically nonlinear least squares algorithm, based on an experimental data set. By means of the optimized model, an adaptive Luenberger observer is built to estimate online the SoC of the lithium-ion battery pack. The observer gain is adaptively adjusted using a stochastic gradient approach so as to reduce the error between the estimated battery output voltage and the filtered battery terminal voltage measurement. Validation results show that the proposed technique can accurately estimate SoC of the lithium-ion battery pack without a heavy computational load.

  19. Charge state effect on Si K X-ray emission induced by Iq+ ions impacting

    Science.gov (United States)

    Lei, Yu; Zhao, Yongtao; Cheng, Rui; Zhou, Xianming; Sun, Yuanbo; Wang, Xing; Wang, Yuyu; Ren, Jieru; Li, Yongfeng; Yu, Yang; Liu, Shidong; Xu, Ge

    2014-04-01

    K X-ray emission of Si induced by Iq+ (q=20, 22, 25) ion impact has been investigated. The results show a much higher intensity of X-ray emission for I25+ ions bombardment compared to I20+ and I22+ ions. The experimental data are explained within the framework of 3dπ, δ-3dσ rotational coupling.

  20. Influence of multi-electron charge-changing processes on the average charge states of heavy ions passing through a He-gas target

    International Nuclear Information System (INIS)

    Average (equilibrium) charge states q¯ of heavy Acq+ (Z = 89), Noq+ (Z = 102) and Flq+ (Z = 114) ions passing through a He-gas target at energies 50–150 keV/u are calculated with account for single- and multi-electron loss and capture cross sections. The q¯ values are obtained by solving the balance equations for equilibrium charge-state fractions and using single-, double- and triple-electron loss cross sections and single- and double-electron capture cross sections. Calculations of all electron-loss and single-capture cross sections are performed using available computer codes, and double-electron capture cross sections are estimated using a new semi-empirical formula obtained in this work on the basis of available experimental data for He target atoms. The account for the multi-electron processes changes significantly (up to about 25%) the q¯ values compared with those calculated with only single-electron cross sections and leads to a better agreement with experimental data

  1. A method for state-of-charge estimation of Li-ion batteries based on multi-model switching strategy

    International Nuclear Information System (INIS)

    Highlights: • Build a multi-model switching SOC estimate method for Li-ion batteries. • Build an improved interpretative structural modeling method for model switching. • The feedback strategy of bus delay is applied to improve the real-time performance. • The EKF method is used for SOC estimation to improve the estimated accuracy. - Abstract: The accurate state-of-charge (SOC) estimation and real-time performance are critical evaluation indexes for Li-ion battery management systems (BMS). High accuracy algorithms often take long program execution time (PET) in the resource-constrained embedded application systems, which will undoubtedly lead to the decrease of the time slots of other processes, thereby reduce the overall performance of BMS. Considering the resource optimization and the computational load balance, this paper proposes a multi-model switching SOC estimation method for Li-ion batteries. Four typical battery models are employed to build a close-loop SOC estimation system. The extended Kalman filter (EKF) method is employed to eliminate the effect of the current noise and improve the accuracy of SOC. The experiments under dynamic current conditions are conducted to verify the accuracy and real-time performance of the proposed method. The experimental results indicate that accurate estimation results and reasonable PET can be obtained by the proposed method

  2. Production and ion-ion cooling of highly charged ions in electron string ion source.

    Science.gov (United States)

    Donets, D E; Donets, E D; Donets, E E; Salnikov, V V; Shutov, V B; Syresin, E M

    2009-06-01

    The scheme of an internal injection of Au atoms into the working space of the "Krion-2" electron string ion source (ESIS) was applied and tested. In this scheme Au atoms are evaporated from the thin tungsten wire surface in vicinity of the source electron string. Ion beams with charge states up to Au51+ were produced. Ion-ion cooling with use of C and O coolant ions was studied. It allowed increasing of the Au51+ ion yield by a factor of 2. Ions of Kr up to charge state 28+ were also produced in the source. Electron strings were first formed with injection electron energy up to 6 keV. Methods to increase the ESIS ion output are discussed. PMID:19566200

  3. Detection method for dissociation of multiple-charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Smith, Richard D. (Richland, WA); Udseth, Harold R. (Richland, WA); Rockwood, Alan L. (Richland, WA)

    1991-01-01

    Dissociations of multiple-charged ions are detected and analyzed by charge-separation tandem mass spectrometry. Analyte molecules are ionized to form multiple-charged parent ions. A particular charge parent ion state is selected in a first-stage mass spectrometer and its mass-to-charge ratio (M/Z) is detected to determine its mass and charge. The selected parent ions are then dissociated, each into a plurality of fragments including a set of daughter ions each having a mass of at least one molecular weight and a charge of at least one. Sets of daughter ions resulting from the dissociation of one parent ion (sibling ions) vary in number but typically include two to four ions, one or more multiply-charged. A second stage mass spectrometer detects mass-to-charge ratio (m/z) of the daughter ions and a temporal or temporo-spatial relationship among them. This relationship is used to correlate the daughter ions to determine which (m/z) ratios belong to a set of sibling ions. Values of mass and charge of each of the sibling ions are determined simultaneously from their respective (m/z) ratios such that the sibling ion charges are integers and sum to the parent ion charge.

  4. Gaseous charge transfer reactions of multiply charged ions

    International Nuclear Information System (INIS)

    Doubly charged ions produced in electron impact ionization have received relatively little study due to their low abundance and masking from singly charged ions which are detected at the same mass-to-charge ratio by a mass spectrometer. This interference problem was avoided by exploiting a technique in which doubly charged molecular and fragment ions are monitored using a collisional charge-exchange process where only fast singly charged product ions are allowed to reach the detector. Primary research efforts were to determine structures and energetics of multiply charged ions formed in high energy electron impact ionization processes and their reactivities in ion-molecule charge exchange interactions. Doubly charged ion mass distributions for various chemical classes (including acetylenes, alkenes, terpenes and organophosphorus compounds) were recorded and appearance energies of prominent doubly charged ions were measured. Computer molecular orbital calculations (at the MINDO/3 level) of ionic structures, energies and charge distributions were utilized to augment the analysis of experimental results

  5. Design of a 2.45 GHz ECR Ion Source for Production of Medium Charge States Ions

    International Nuclear Information System (INIS)

    At Lawrence Berkeley National Laboratory we are constructing an ECR ion source test facility for nuclear science experiments. For this purpose a single-stage 2.45 GHz electron cyclotron resonance ion source has been designed and fabricated. It features an axial magnetic field with a mirror ratio of up to 5.5 and a hexapole field produced by a novel Nd-Fe-B permanent magnet assembly. In order to enhance the ion confinement time the source plasma volume has been enlarged as much as possible while still maintaining a high mirror ratio. This paper describes the design of the source. Ion optics simulation of the extraction system currently under design will also be presented

  6. Acceleration and Utilization of Highly Stripped Charge State Heavy Ions at HI-13 Acceleration

    Institute of Scientific and Technical Information of China (English)

    2002-01-01

    Even higher linear energy transfer (LET) values of the heavy ions are necessary as the investigationsof single event effects (SEE) of satellite devices are developing rapidly. For example, the researches aredeveloped from the single-event upset (SEU) which needs comparatively low LET values towards singleevent latch up (SEL) and single event burnout (SEB) which requires high LET values, namely LET’s arehigher than 80 MeV mg-1,cm-2 and range of the ions in the silicon should be large than 20 micrometers,

  7. An integrated approach for real-time model-based state-of-charge estimation of lithium-ion batteries

    Science.gov (United States)

    Zhang, Cheng; Li, Kang; Pei, Lei; Zhu, Chunbo

    2015-06-01

    Lithium-ion batteries have been widely adopted in electric vehicles (EVs), and accurate state of charge (SOC) estimation is of paramount importance for the EV battery management system. Though a number of methods have been proposed, the SOC estimation for Lithium-ion batteries, such as LiFePo4 battery, however, faces two key challenges: the flat open circuit voltage (OCV) vs SOC relationship for some SOC ranges and the hysteresis effect. To address these problems, an integrated approach for real-time model-based SOC estimation of Lithium-ion batteries is proposed in this paper. Firstly, an auto-regression model is adopted to reproduce the battery terminal behaviour, combined with a non-linear complementary model to capture the hysteresis effect. The model parameters, including linear parameters and non-linear parameters, are optimized off-line using a hybrid optimization method that combines a meta-heuristic method (i.e., the teaching learning based optimization method) and the least square method. Secondly, using the trained model, two real-time model-based SOC estimation methods are presented, one based on the real-time battery OCV regression model achieved through weighted recursive least square method, and the other based on the state estimation using the extended Kalman filter method (EKF). To tackle the problem caused by the flat OCV-vs-SOC segments when the OCV-based SOC estimation method is adopted, a method combining the coulombic counting and the OCV-based method is proposed. Finally, modelling results and SOC estimation results are presented and analysed using the data collected from LiFePo4 battery cell. The results confirmed the effectiveness of the proposed approach, in particular the joint-EKF method.

  8. Enhanced closed loop State of Charge estimator for lithium-ion batteries based on Extended Kalman Filter

    International Nuclear Information System (INIS)

    Highlights: • Based on a general model valid in full range of SOC considering varied dynamics. • Integration of an accurate OCV model in EKF taking into account hysteresis effect. • Experimental validation with different current profiles: pulses, EV and lift. • Validated with specifically designed profile demanding accurate OCV modeling. - Abstract: The accurate State of Charge (SOC) estimation in a Li-ion battery requires a suitable model of the cell behavior. In this work an enhanced closed loop estimator based on Extended Kalman Filter (EKF) is proposed, considering a precise model of the cell dynamics valid for different current profiles and SOCs, and a complete model of the Open Circuit Voltage (OCV) which takes into account the hysteresis influence. The employed model and proposed estimator are validated with experimental results obtained from the response of a 40 Ah NMC Li-ion cell to several current profiles. These tests include current pulses, FUDS driving cycles, residential lift profiles, and specially designed profiles which demand an accurate modeling of the transitions between OCV boundaries. In each case, it is demonstrated that the enhanced model can reduce the estimation error nearly by half compared to an estimator ignoring the hysteresis effect. Furthermore, the good performance of the cell dynamics model allows an accurate and stable estimation over different conditions

  9. HICS: Highly charged ion collisions with surfaces

    CERN Document Server

    Peters, Thorsten; Hopster, Johannes; Sokolovsky, Valentin; Wucher, Andreas; Schleberger, Marika

    2008-01-01

    The layout of a new instrument designed to study the interaction of highly charged ions with surfaces, which consists of an ion source, a beamline including charge separation and a target chamber, is presented here. By varying the charge state and impact velocity of the projectiles separately, the dissipation of potential and kinetic energy at or below the surface can be studied independently. The target chamber offers the use of tunable metal-insulator-metal devices as detectors for internal electronic excitation, a timeof-flight system to study the impact induced particle emission and the possibility to transfer samples in situ to a UHV scanning probe microscope. Samples and detectors can be prepared in situ as well. As a first example data on graphene layers on SrTiO3 which have been irradiated with Xe36+ are presented. Key words: highly charged ions, sputtering, AFM, graphene

  10. Highly charged ions trapping for lifetime measurements

    International Nuclear Information System (INIS)

    A new experimental setup dedicated to highly charged ion trapping is presented in this work. The final goal is to perform lifetime measurement of metastable states produced by our ECR (Electron Cyclotron Resonance) ion source. Lifetimes to be measured are in the range of a few ms and more. We have measured the lifetimes of the M1 transitions of the metastable states of Ar9+, Ar13+ and Ar14+. These measurements are useful to test the N-body problem in the relativistic range. The trap we have built, was designed a few years ago at the Weizman Institute in Israel, it allows ions with an energy of several keV to be trapped for lifetimes of about 1 second. This trap was originally designed to study the dynamics of excited molecules. We have shown for the first time how the trap operates and that it can operate with highly charged ions. We have studied the beam dynamics of highly charged ions and the trap has been tested with various species of ions and different charge states: from O+ to O6+, from Ar8+ to Ar13+, and from Kr13+ to Kr20+

  11. Ionization cross sections of state selective atomic hydrogen by impact of multiply charged ions

    International Nuclear Information System (INIS)

    Ionization cross sections of atomic hydrogen in ground state and in metastable 2s state in collision with bare projectiles over a wide energy range have been calculated. The final state wave function considers the distortion due to Coulomb fields of both the projectile and the target nucleus. The present calculated total ionization cross-section values show good accord with the measurements for He2+, Li3- and C6+ impact at intermediate and high energy region. (author)

  12. The charge state distributions of 0.5-2.9 MeV Be, Al, Cl, Ti and Ni ions measured after carbon foil stripping

    International Nuclear Information System (INIS)

    Equilibrium charge state distributions have been measured for Be, Al, Cl, Ti and Ni ions stripped in the high-voltage terminal of an electrostatic tandem accelerator using a 2 μg/cm2 carbon foil. The series of measurements were made with a terminal voltage ranging from typically 1.5 to 2.9 MV. The charge state distributions were measured on the high-energy side of the accelerator, just in front of the analysing magnet, in order to take charge state-dependent transmission through the high-energy side of the accelerator into account. The obtained charge state distributions will be used for accelerator mass spectrometry measurements to find the optimum terminal voltage of the accelerator. (orig.)

  13. Abundances, charge states, and energy spectra of helium and heavy ions during solar particle events

    Science.gov (United States)

    Gloeckler, G.; Sciambi, R.; Fan, C. Y.; Hovestadt, D.

    1975-01-01

    Carbon and oxygen energy spectra observed during several solar events indicate a systematic deviation of these spectra from a simple power law: the spectra bend down below about 100 keV/nuc and the amount of this bending is highly correlated with the size of the flare, as measured by the 'event averaged' flux of 130-220 keV protons. The energy spectra of helium computed for the same time periods do not show a similar feature. A large variability of the alpha/CNO ratio is found from event to event (from 2 to about 20 at 40 keV/nuc), and in all cases examined the carbon and oxygen nuclei are nearly fully stripped. These results are interpreted as evidence for storage of energetic ions in hot coronal regions, followed by strong adiabatic deceleration.

  14. A Combined State of Charge Estimation Method for Lithium-Ion Batteries Used in a Wide Ambient Temperature Range

    Directory of Open Access Journals (Sweden)

    Fei Feng

    2014-05-01

    Full Text Available Ambient temperature is a significant factor that influences the characteristics of lithium-ion batteries, which can produce adverse effects on state of charge (SOC estimation. In this paper, an integrated SOC algorithm that combines an advanced ampere-hour counting (Adv Ah method and multistate open-circuit voltage (multi OCV method, denoted as “Adv Ah + multi OCV”, is proposed. Ah counting is a simple and general method for estimating SOC. However, the available capacity and coulombic efficiency in this method are influenced by the operating states of batteries, such as temperature and current, thereby causing SOC estimation errors. To address this problem, an enhanced Ah counting method that can alter the available capacity and coulombic efficiency according to temperature is proposed during the SOC calculation. Moreover, the battery SOCs between different temperatures can be mutually converted in accordance with the capacity loss. To compensate for the accumulating errors in Ah counting caused by the low precision of current sensors and lack of accurate initial SOC, the OCV method is used for calibration and as a complement. Given the variation of available capacities at different temperatures, rated/non-rated OCV–SOCs are established to estimate the initial SOCs in accordance with the Ah counting SOCs. Two dynamic tests, namely, constant- and alternated-temperature tests, are employed to verify the combined method at different temperatures. The results indicate that our method can provide effective and accurate SOC estimation at different ambient temperatures.

  15. An Adaptive Gain Nonlinear Observer for State of Charge Estimation of Lithium-Ion Batteries in Electric Vehicles

    Directory of Open Access Journals (Sweden)

    Yong Tian

    2014-09-01

    Full Text Available The state of charge (SOC is important for the safety and reliability of battery operation since it indicates the remaining capacity of a battery. However, it is difficult to get an accurate value of SOC, because the SOC cannot be directly measured by a sensor. In this paper, an adaptive gain nonlinear observer (AGNO for SOC estimation of lithium-ion batteries (LIBs in electric vehicles (EVs is proposed. The second-order resistor–capacitor (2RC equivalent circuit model is used to simulate the dynamic behaviors of a LIB, based on which the state equations are derived to design the AGNO for SOC estimation. The model parameters are identified using the exponential-function fitting method. The sixth-order polynomial function is used to describe the highly nonlinear relationship between the open circuit voltage (OCV and the SOC. The convergence of the proposed AGNO is proved using the Lyapunov stability theory. Two typical driving cycles, including the New European Driving Cycle (NEDC and Federal Urban Driving Schedule (FUDS are adopted to evaluate the performance of the AGNO by comparing with the unscented Kalman filter (UKF algorithm. The experimental results show that the AGNO has better performance than the UKF algorithm in terms of reducing the computation cost, improving the estimation accuracy and enhancing the convergence ability.

  16. Influence of incident charge state of fast ion (Pb{sup n+} at 4.6 MeV/u) on the secondary emission from mica surface; Influence de la charge incidente d`ion rapide (Pb{sup n+} A 4.6 MeV/u) sur l`emission secondaire sur une surface de mica

    Energy Technology Data Exchange (ETDEWEB)

    Brunelle, A.; Della-Negra, S.; Depauw, J.; Jacquet, D. [Experimental Research Division, Inst. de Physique Nucleaire, Paris-11 Univ., 91 - Orsay (France); Rozet, J.P.; Vernhet, D. [GPS-PIIM, Paris-6 Univ., 75 - Paris (France); Bouffard, S.; Cassimi, A.; Gervais, B.; Grandin, J.P.; Leroy, C.; Rothard, H.; Buve, M. [CIRIL, Caen Univ., 14 - Caen (France)

    1999-11-01

    The damage induced by heavy ion in the mica has been studied. The first quantitative results allowed by atomic force microscopy realized at CIRIL on mica samples irradiated by fast heavy ions have shown clearly a dependence on the incident charge state. The evolution of track diameters with ion charge states presents a step-like behaviour with 2 plateaus on both sides of the equilibrium charge states. The secondary ion emission studied in the same experimental conditions shows that the ions emitted from the mica are not sensitive to the same phenomena like those involved in the damage creation. The secondary ion yields do not follow the same charge state dependence. (authors) 5 refs., 2 figs.

  17. The Kansas State atomic collision physics facility dedicated to the studies of atomic interactions of highly charged, low and medium energy ions

    International Nuclear Information System (INIS)

    We discuss our facility at Kansas State University, which is perfectly suited for studies of atomic collisions involving highly charged, low and medium energy ions. It should be fully operational by next year and will be operated as a user facility. We encourage collaborations with in-house researchers, because it facilitates communications and experiments. 13 refs., 3 figs

  18. Proposed precision laser spectrometer for trapped, highly charged ions

    OpenAIRE

    M. Vogel; Winters, D.F.A.; Segal, D. M.; Thompson, R. C.

    2005-01-01

    We propose a novel type of precision laser spectrometer for trapped, highly charged ions nearly at rest. It consists of a cylindrical open-endcap Penning trap in which an externally produced bunch of highly charged ions can be confined and investigated by means of laser spectroscopy. The combination of confinement, cooling and compression of a dense ion cloud will allow the ground state hyperfine splitting in highly charged ions to be measured with an accuracy three orders of magnitude better...

  19. Absolute differential and total cross sections for charge transfer of O{sup +} ground and mixed states ions in N{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Martinez, H [Centro de Ciencias Fisicas, Universidad Nacional Autonoma de Mexico, Cuernavaca, Morelos, PO Box 48-3, 62251, Cuernavaca, Morelos (Mexico); Hernandez, C L [Centro de Ciencias Fisicas, Universidad Nacional Autonoma de Mexico, Cuernavaca, Morelos, PO Box 48-3, 62251, Cuernavaca, Morelos (Mexico); Yousif, F B [Facultad de Ciencias, Universidad Autonoma del Estado de Morelos, Avenida Universidad 1001, 62210, Cuernavaca, Morelos (Mexico)

    2006-06-14

    We report measurements of the total and absolute differential cross sections for charge transfer of ground- and excited-states O{sup +} ions at 1.0, 1.5, 2.0, 2.5, 3.0, 3.5, 4.0, 4.5 and 5 keV in collisions with N{sub 2} at scattering angles -5.2{sup 0} {<=} {theta} {<=} +5.2{sup 0} in the laboratory frame. Total cross sections for ground- and mixed state ions are compared with previous measurements. The behaviour of the absolute differential cross sections display an expected decreasing behaviour with increasing angle. The mixed state ions cross sections are considerably higher than those measured for the ground state ions.

  20. Vibrationally state selected ion molecule experimental and computational studies of both reactant charge states of [nitrogen dioxide + ethyne]+ and HOD+ with nitrogen dioxide

    Science.gov (United States)

    Boyle, Jason M.

    2011-12-01

    Ion molecule studies have not only determined reactivity of systems that would have otherwise been unavailable, but also provide a perspective that improves the understanding of the mechanisms that drive reaction. Presented here are studies of three ion molecule systems one of which is accompanied by an extensive set of direct dynamics trajectory calculations. In the first system presented, NO2+ in six different vibrational states was reacted with C2H2 over the center-of-mass energy range from 0.03 to 3.3 eV. The effects of the symmetric bend overtone (0200) excitation are particularly strong (factor of 4) while the delta overtone (0220) effects are much weaker. A large set of quasi-classical trajectories were calculated at the PBE1PBE/6-311G** level of theory, in an attempt to understand the mechanistic origins of this observation. The trajectories reproduce experiment where comparable. Analysis of these trajectories resolves the mechanistic origins of this vibrational effect. Similar experimental measurements were made for the first excited electronic state of this system where the charge is localized on the acetylene. The C 2H2+ reactant was prepared in four distinct modes. Because both reactants have one unpaired electron, collisions can occur with either singlet or triplet coupling of these unpaired electrons, and the contributions the three channels (charge, O-, and O transfer) are separated based on distinct recoil dynamics. The effects of C2H 2+ vibration are modest, but mode specific. Integral cross sections and product recoil velocity distributions were also measured for reaction of HOD+ with NO2, in which the HOD+ reactant was prepared in its ground state, and with mode-selective excitation in the 001 (OH stretch), 100 (OD stretch) and bend (010) modes. In addition, we measured the 300 K thermal kinetics in a selected ion flow tube reactor and report product branching ratios different from previous measurements. Reaction is found to occur on both the

  1. Charge-state dependence of M-shell x-ray production in 67Ho by 2--12-MeV carbon ions

    International Nuclear Information System (INIS)

    Charge-state dependence of M-shell x-ray production cross sections of 67Ho bombarded by 2--12-MeV carbon ions, with and without K-shell vacancies, were measured using a windowless Si(Li) x-ray detector with a full-width-at-half-maximum resolution of 135 eV at 5.9 keV. Carbon ions of different charge states were produced using a postacceleration, nitrogen gas stripping cell. The carbon ions were then magnetically analyzed to select the desired charge state and energy before entering the target chamber. The total M-shell and Mζ, Mα,β, and Mγ x-ray cross sections were measured. The electron-capture (EC) contributions as well as the direct-ionization (DI) contributions can be determined by making a comprehensive study of the projectile-charge-state dependence of the target x-ray production cross sections for targets in which the single-collision realm is maintained. In this paper, both EC and DI contributions and the total M-shell x-ray production cross sections are compared to both the first Born theory and to the perturbed-stationary-state theory with energy-loss, Coulomb-deflection, and relativistic corrections

  2. Evaluation of Lithium-Ion Battery Equivalent Circuit Models for State of Charge Estimation by an Experimental Approach

    Directory of Open Access Journals (Sweden)

    Jinxin Fan

    2011-03-01

    Full Text Available To improve the use of lithium-ion batteries in electric vehicle (EV applications, evaluations and comparisons of different equivalent circuit models are presented in this paper. Based on an analysis of the traditional lithium-ion battery equivalent circuit models such as the Rint, RC, Thevenin and PNGV models, an improved Thevenin model, named dual polarization (DP model, is put forward by adding an extra RC to simulate the electrochemical polarization and concentration polarization separately. The model parameters are identified with a genetic algorithm, which is used to find the optimal time constant of the model, and the experimental data from a Hybrid Pulse Power Characterization (HPPC test on a LiMn2O4 battery module. Evaluations on the five models are carried out from the point of view of the dynamic performance and the state of charge (SoC estimation. The dynamic performances of the five models are obtained by conducting the Dynamic Stress Test (DST and the accuracy of SoC estimation with the Robust Extended Kalman Filter (REKF approach is determined by performing a Federal Urban Driving Schedules (FUDS experiment. By comparison, the DP model has the best dynamic performance and provides the most accurate SoC estimation. Finally, sensitivity of the different SoC initial values is investigated based on the accuracy of SoC estimation with the REKF approach based on the DP model. It is clear that the errors resulting from the SoC initial value are significantly reduced and the true SoC is convergent within an acceptable error.

  3. Nanodots formation with slow highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Yamazaki, Yasunori [Graduate School of Arts and Sciences, University of Tokyo and RIKEN (Japan)

    2007-06-15

    We have been developing a compact electron beam ion source with a high-T{sub c}superconductor as a solenoid magnet, which can be operated at liquid nitrogen temperature, and can deliver slow highly-charged ions as high as q 42. With this ion source together with other ion sources, nanodot formation processes were studied for a highly oriented pyrolytic graphite (HOPG) plate as a target. The impact site was observed with both the scanning tunnelling microscope (STM) mode and non-contact atomic force microscope (NCAFM) mode. It was found that protrusion-like dots were observed for both modes at the same position, and one HCI induced one dot. The dot size (diameter) and height were observed to be more or less the same for both modes, i.e, an HCI impact induces topographic modification on the HOPG surface. The dot size and height were measured as functions of the charge state (q = 8-46) and the kinetic energy (E = 1-300 keV) of highly-charged ions. It was found that the dot size increased linearly with the charge state, although the dependence on the kinetic energy was very weak if any.

  4. Improved phenomenological description of equilibrium charge state distributions for Ni, Co, and Cu ions in Mo based on new experimental data at 2 MeV/u

    CERN Document Server

    Gastis, P; Robertson, D; Almus, R; Anderson, T; Bauder, W; Collon, P; Lu, W; Ostdiek, K; Skulski, M

    2015-01-01

    Equilibrium charge state distributions of stable 60Ni, 59Co, and 63Cu beams passing through a 1um thick Mo foil were measured at beam energies of 1.84 MeV/u, 2.09 MeV/u, and 2.11 MeV/u respectively. A 1-D position sensitive Parallel Grid Avalanche Counter detector (PGAC) was used at the exit of a spectrograph magnet, enabling us to measure the intensity of several charge states simultaneously. The number of charge states measured for each beam constituted more than 99% of the total equilibrium charge state distribution for that elements. Currently, little experimental data exists for equilibrium charge state distributions for heavy ions with 19charge states and distribution widths), has not been thoroughly tested at the energy region of interest. A number of semi-empirical models from the literature were evalu...

  5. Heavy Coronal Ions in the Heliosphere: I. Global Distribution of Charge-states of C, N, O, Mg, Si and S

    CERN Document Server

    Grzedzielski, S; Bzowski, M; Izmodenov, V

    2008-01-01

    Aims: Investigate/Study de-charging of solar wind C, N, O, Mg, Si and S ions and assess fluxes of resulting ENA in the heliosphere. Methods: The model treats the heavy ions as test particles convected by (and in a particular case also diffusing through) a hydrodynamically calculated background plasma flow, from 1 AU to the termination shock (TS), to heliosheath (HS) and finally to heliospheric tail (HT). The ions undergo radiative and dielectronic recombinations, charge exchanges, photo- and electron impact ionizations with plasma particles, interstellar neutral atoms (calculated on a Monte-Carlo model) and solar photons. Results: Highly-charged heavy coronal ions flowing with the solar wind undergo successive de-ionizations, mainly in the heliosheath, leading to charge-states much lower than in the supersonic solar wind. If Coulomb scattering is the main ion energy loss mechanism, the end product of these deionizations are fluxes of ENA of ~1 keV/nucleon originating in the upwind heliosheath that for C, Mg, ...

  6. Results from E-Mevva and Z-Mevva: Development of new sources of intense high charge state heavy-ion beams

    International Nuclear Information System (INIS)

    The authors are exploring a new approach for heavy ion beam injection (e.g., into the Relativistic Heavy Ion Collider (RHIC) at BNL), as well as new sources of intense high charge state ions to be mounted on a relatively low voltage platform for high energy ion implantation. While conventional Metal Vapor Vacuum Arc (Mevva) ion sources can produce up to hundreds of milliamps or more of several-times-ionized metal ions (e.g., U3+), the recent results from Batalin et al. indicate that the addition of an energetic electron beam (E-Mevva) may lead to considerably higher charge states. An alternative way to produce the electron beam is Z-Mevva, in which a z-discharge plasma is used to enhance multiple ionization. As the vacuum arc plasma plume expands into a magnetized drift region, a z-discharge is triggered in the drifting metal plasma. The ions are then extracted and analyzed using a time-of-flight system. The authors report initial results using these schemes with applied discharge and electron beam voltages from 1 to 2 kV

  7. A data-driven based adaptive state of charge estimator of lithium-ion polymer battery used in electric vehicles

    International Nuclear Information System (INIS)

    Highlights: • A lumped parameter battery model against different battery aging levels is proposed. • The RLS based method is used to identify the parameter of battery model in real-time. • A data-driven based adaptive SoC estimator is developed by RLS and AEKF algorithm. • The robustness of the SoC estimator against varying loading profiles is evaluated. • The robustness of the SoC estimator against different aging levels is evaluated. - Abstract: An accurate State of Charge (SoC) estimation method is one of the most significant and difficult techniques to promote the commercialization of electric vehicles. The paper attempts to make three contributions. (1) Through the recursive least square algorithm based identification method, the parameter of the lumped parameter battery model can be updated at each sampling interval with the real-time measurement of battery current and voltage, which is called the data-driven method. Note that the battery model has been improved with a simple electrochemical equation for describing the open circuit voltage against different aging levels and SoC. (2) Through the real-time updating technique of model parameter, a data-driven based adaptive SoC estimator is established with an adaptive extended Kalman filter. It has the potential to overcome the estimation error against battery degradation and varied operating environments. (3) The approach has been verified by different loading profiles of various health states of Lithium-ion polymer battery (LiPB) cells. The results indicate that the maximum estimation errors of voltage and SoC are less than 1% and 1.5% respectively

  8. Equilibrium and non-equilibrium charge-state distributions of 2 MeV/u sulfur ions passing through carbon foils

    International Nuclear Information System (INIS)

    Both equilibrium and non-equilibrium charge-state distributions for 2.0 MeV/u sulfur ions after passing through carbon foils were studied experimentally. For the equilibrium charge-state distribution, incident ions of S7+, S12+, S14+ and S16+ were injected into carbon foils 54, 98, 150 and 200 μg/cm2 in thickness, whereas for the non-equilibrium distributions, new measurements for S15+ and S16+ incidences were made through carbon foils of 0.9-10 μg/cm2 to supplement our previous experiments regarding S6+-S14+ incidences [M. Imai, M. Sataka, K. Kawatsura, K. Takahiro, K. Komaki, H. Shibata, H. Sugai, K. Nishio, Nucl. Instr. and Meth. B 230 (2005) 63; M. Imai, M. Sataka, K. Kawatsura, K. Takahiro, K. Komaki, H. Shibata, H. Sugai, K. Nishio, Nucl. Instr. and Meth. B 256 (2007) 11]. Mean charge states for S6+-S14+ incidences as functions of the penetration thickness merged at 6.9 μg/cm2 and changed together until reaching equilibrium at around 100 μg/cm2, while those for S15+ and S16+ incidences took different paths to equilibrium, which was also the case for distribution widths for S6+-S14+, S15+ and S16+ incidences. An equilibrium mean charge state of 12.68 and distribution width of 1.11 were attained with equilibrium charge distributions between 6+ and 16+.

  9. Charge-state and energy enhancment of laser-produced ions due to nonlinear processes in performed plasma

    Czech Academy of Sciences Publication Activity Database

    Láska, Leoš; Jungwirth, Karel; Krása, Josef; Pfeifer, Miroslav; Rohlena, Karel; Ullschmied, Jiří; Badziak, J.; Parys, P.; Wolowski, J.; Gammino, S.; Torrisi, L.; Boody, F. P.

    2005-01-01

    Roč. 86, č. 8 (2005), 081502/1-081502/3. ISSN 0003-6951 R&D Projects: GA AV ČR(CZ) IAA1010405; GA MŠk(CZ) LN00A100; GA AV ČR(CZ) KSK2043105 Institutional research plan: CEZ:AV0Z10100523 Keywords : laser-beam interaction * non-linear processes * highly - charged ions Subject RIV: BH - Optics, Masers, Lasers Impact factor: 4.127, year: 2005

  10. Charge density at the nucleus and radial behavior of ground state for lithium-like ions with Z =21 to 30

    Institute of Scientific and Technical Information of China (English)

    Yu Wei-Wei; Wang Zhi-Wen; Chen Chao; Cai Juan; Zhang Nan

    2012-01-01

    By using the full-core plus correlation (FCPC) type wave functions,the accurate charge densities ρ(0) at the nucleus and the radial expectation values of the ground states for the lithium-like systems with Z =21 to 30 are obtained.The determinantal conditious and the electron-nucleus cusp condition are used to calculate the inequalities of the upper and the lower bounds to ρ(0) with two or more expectation values.These inequalities,derived by Angulo and Dehesa [Phys.Rev.A 44 1516 (1991)],are verified to be also valid for these ions with higher nuclear charge.The present results show that the wave functions used in this paper are satisfactory in the whole configuration space for these ions with higher nuclear charge.

  11. Energy loss and charge state distribution of calcium ions in dense moderately coupled carbon plasma; Energieverlust und Ladungsverteilung von Calciumionen in dichtem, schwach gekoppeltem Kohlenstoffplasma

    Energy Technology Data Exchange (ETDEWEB)

    Ortner, Alex

    2015-07-15

    In this thesis the interaction of swift calcium ions (Energy: 3.5 MeV/u) with a dense and moderately coupled carbon plasma (Coupling parameter: Γ=0.1-0.5) is investigated. The plasma state is generated by heating a thin carbon foil volumetrically by thermal X-ray radiation. The thermal X-ray radiation itself is generated by the conversion of a high energy laser beam in a hohlraum cavity. Compared to earlier ion stopping experiments the electron density and the plasma coupling parameter could be increased by an order of magnitude. This work provides the first time experimental energy loss and charge state distribution data in this moderately coupled interaction regime. The thesis consists of a theoretical part where the ion beam plasma interaction is studied for a broad range of plasma parameters and an experimental part where the ion beam interaction with the hohlraum plasma target is measured. All the described experiments were carried out at the GSI Helmholtzzentrum fuer Schwerionenforschung in Darmstadt. This facility offers the unique possibility to combine a heavy ion beam from an accelerator with a high energy laser beam in one interaction chamber. An intense laser pulse (150 J of laser energy in 1 ns at λ{sub L}=527 nm) is focused inside a 600 μm diameter spherical cavity and generates a hot gold plasma that emits X-rays. The absorbed and reemitted radiation establishes a spatially uniform temperature distribution in the cavity and serves as an intense, isotropic X-ray source with a quasi-thermal spectral distribution. These thermal X-rays with a radiation temperature of T{sub r}=98±6 eV then propagate into a secondary cylindrical hohlraum (diameter: 1000 μm, length: 950 μm) where they volumetrically heat two thin carbon foils to the plasma state. The radiation temperature in the secondary hohlraum is T{sub r}=33±5 eV. This indirect laser heating scheme has the advantage that the whole sample volume is instantaneously heated and that the plasma is

  12. Adiabatic calorimetry test of the reaction kinetics and self-heating model for 18650 Li-ion cells in various states of charge

    Science.gov (United States)

    Chen, Wei-Chun; Wang, Yih-Wen; Shu, Chi-Min

    2016-06-01

    Use of adiabatic calorimetry to characterise thermal runaway of Li-ion cells is a crucial technique in battery safety testing. Various states of charge (SoC) of Li-ion cells were investigated to ascertain their thermal runaway features using a Vent Sizing Package 2 (VSP2) adiabatic calorimeter. To evaluate the thermal runaway characteristics, the temperature-pressure-time trajectories of commercial cylindrical cells were tested, and it was found that cells at a SoC of greater than 50% were subject to thermal explosion at elevated temperatures. Calorimetry data from various 18650 Li-ion cells with different SoC were used to calculate the thermal explosion energies and chemical kinetics; furthermore, a novel self-heating model based on a pseudo-zero-order reaction that follows the Arrhenius equation was found to be applicable for studying the exothermic reaction of a charged cell.

  13. Excited state charge transfer reaction in (mixed solvent + electrolyte) systems: Role of reactant-solvent and reactant-ion interactions

    Indian Academy of Sciences (India)

    Harun Al Rasid Gazi; Ranjit Biswas

    2011-05-01

    Fluorescence spectroscopic techniques have been used to study the excited state intramolecular charge transfer reaction of 4-(1-azetidinyl)benzonitrile (P4C) in two sets of mixed solvents, (1-propanol + ethyl acetate) and (propylene carbonate + acetonitrile), in the absence and presence of a strong electrolyte, lithium perchlorate. These two sets of mixed solvent systems represent binary solvent mixtures of low and high polarities, respectively. Density, sound velocity and viscosity measurements indicate that these two mixed solvent systems are structurally different. Stronger ion-reactant interaction is evidenced in the mole fraction independence of emission frequencies in electrolyte solutions of low polar binary solvent mixtures. For both these mixtures, the reaction driving force (- ) decreases with increase in mole fraction of the relatively less polar solvent component of the mixture. Interestingly, - increases significantly on addition of electrolyte in low polar mixtures and exhibits mixture composition dependence but, in contrast, - in high polar mixtures does not sense variation in mixture composition in presence of electrolyte. This insensitivity to mixture composition for high polar mixtures is also observed for the measured reaction time constant. In addition, the reaction time constant does not sense the presence of electrolyte in the high polar solvent mixtures. The reaction time constant in low polar mixtures, which becomes faster on addition of electrolyte, lengthens on increasing the mole fraction of the relatively less polar solvent component of the mixture. These observations have been qualitatively explained in terms of the measured solvent reorganization energy and reaction driving force by using expressions from the classical theory of electron transfer reaction.

  14. Novel Energy Sources -Material Architecture and Charge Transport in Solid State Ionic Materials for Rechargeable Li ion Batteries

    Energy Technology Data Exchange (ETDEWEB)

    Katiyar, Ram S; Gómez, M; Majumder, S B; Morell, G; Tomar, M S; Smotkin, E; Bhattacharya, P; Ishikawa, Y

    2009-01-19

    Since its introduction in the consumer market at the beginning of 1990s by Sony Corporation ‘Li-ion rechargeable battery’ and ‘LiCoO2 cathode’ is an inseparable couple for highly reliable practical applications. However, a separation is inevitable as Li-ion rechargeable battery industry demand more and more from this well serving cathode. Spinel-type lithium manganate (e.g., LiMn2O4), lithium-based layered oxide materials (e.g., LiNiO2) and lithium-based olivine-type compounds (e.g., LiFePO4) are nowadays being extensively studied for application as alternate cathode materials in Li-ion rechargeable batteries. Primary goal of this project was the advancement of Li-ion rechargeable battery to meet the future demands of the energy sector. Major part of the research emphasized on the investigation of electrodes and solid electrolyte materials for improving the charge transport properties in Li-ion rechargeable batteries. Theoretical computational methods were used to select electrodes and electrolyte material with enhanced structural and physical properties. The effect of nano-particles on enhancing the battery performance was also examined. Satisfactory progress has been made in the bulk form and our efforts on realizing micro-battery based on thin films is close to give dividend and work is progressing well in this direction.

  15. Inner-shell vacancy production and mean charge states of MeV/u Fe, Co, Ni and Cu ions in Au and Bi solid targets

    International Nuclear Information System (INIS)

    The average charge states of 0.1-1.5 MeV/u Fe, Co, Ni and Cu ions in solid Au and Bi targets have been determined, by estimating the mean numbers of outer-shell spectator vacancies during the K-vacancy decay. The latter quantities were obtained from the yield and energy shifts of the Kα, β X-rays, by comparing with calculations in the independent electron approximation. The reported equilibrium charges, mostly characteristic for the inside of the target, are in fairly agreement with Nikolaev and Dmitriev semi-empirical formula [Phys. Lett. 28A (1968) 277

  16. Kinetic energy and charge state effects in the X-ray emission of Mo surface induced by Xeq+(q=25,29) ions

    Institute of Scientific and Technical Information of China (English)

    2008-01-01

    L-shell X-ray spectra of Mo surface induced by Xe25+ and Xe29+ were measured. The X-ray intensity was obtained in the kinetic energy range of the incident ions from 350 to 600 keV. The relationship of X-ray intensity with kinetic energy of the projec-tile and its charge state were studied,and the simple explanation was given.

  17. Production, transport and charge capture measurements of highly charged recoil ions

    International Nuclear Information System (INIS)

    An experiment is described to study highly charged recoil ions on-line to the heavy ion accelerator UNILAC at GSI. The highly charged recoil ions are produced by heavy ion bombardment of a gas target. Subsequently the slow highly charged recoil ions are extracted from the ionization volume, and guided through a beam transport line to a Wien filter for charge state selection and to a collision region to study charge transfer processes. Several experiments were carried out to show the efficient charge state separation. Charge states up to q=15 were observed. When using a retarding field analyzer cross sections for single electron capture were determined for different charge states of Xeq+ for q=4 to 11 and He gas. The experiments demonstrated increasing charge transfer cross sections with increasing charge state q and indicated the effect of near resonant charge capture for q=6. The flexible data acquisition system used, is described and other future experiments, such as for instance in flight ion-trapping are indicated in the appendix. (orig.)

  18. Modeling of the charge-state separation at ITEP experimental facility for material science based on a Bernas ion source

    International Nuclear Information System (INIS)

    The experiment automation system is supposed to be developed for experimental facility for material science at ITEP, based on a Bernas ion source. The program CAMFT is assumed to be involved into the program of the experiment automation. CAMFT is developed to simulate the intense charged particle bunch motion in the external magnetic fields with arbitrary geometry by means of the accurate solution of the particle motion equation. Program allows the consideration of the bunch intensity up to 1010 ppb. Preliminary calculations are performed at ITEP supercomputer. The results of the simulation of the beam pre-acceleration and following turn in magnetic field are presented for different initial conditions

  19. Modeling of the charge-state separation at ITEP experimental facility for material science based on a Bernas ion source

    Energy Technology Data Exchange (ETDEWEB)

    Barminova, H. Y., E-mail: barminova@bk.ru; Saratovskyh, M. S. [National Research Nuclear University MEPhI, Kashirskoye sh. 31, Moscow 115409 (Russian Federation)

    2016-02-15

    The experiment automation system is supposed to be developed for experimental facility for material science at ITEP, based on a Bernas ion source. The program CAMFT is assumed to be involved into the program of the experiment automation. CAMFT is developed to simulate the intense charged particle bunch motion in the external magnetic fields with arbitrary geometry by means of the accurate solution of the particle motion equation. Program allows the consideration of the bunch intensity up to 10{sup 10} ppb. Preliminary calculations are performed at ITEP supercomputer. The results of the simulation of the beam pre-acceleration and following turn in magnetic field are presented for different initial conditions.

  20. Atomic physics with highly charged ions

    International Nuclear Information System (INIS)

    The past year has been a busy one for all three accelerators, the LINAC, EBIS and the tandem. The EBIS continues to deliver beams of highly charged ions around the clock for the study of low energy collisions with gases and surfaces. The electron beam energy has been upgraded to 10 keV, and intensities of highly charged species such as Xe44+ have been greatly increased. The tandem, the traditional source of highly charged Binary encounter electron production at zero degrees were studied for medium Z (Si,Cl,Cu) projectiles. Recoil momentum spectroscopy has been used to separate the contributions to collisional ionization of one-electron ions (C5+, O7+, F8+) from the nucleus and the electrons of a He target. Marked structure in the binary encounter electron spectra for Cuq+ on H2 targets has been measured for moderate velocity projectiles. Electron capture by slow multiply charged (EBIS) projectiles from laser excited targets has been carried out. Cross sections for capture from Na(3s) and Na*(3p) have been measured for velocities between 0.1 and 1 au. The extension of these experiments to laser excited Rydberg targets is proceeding. Electron capture cross sections and average Q values for Ar16+ on He at velocities between 0.23 and 1.67 au have been measured. The charge state distribution of the He recoils following large angle scattering of C4+ and C6+ ions at 7.5 keV/u has been measured. Cross sections have been measured for up to sextuple capture from C60 (buckminsterfullerene) by highly charged slow projectiles. Coupled channel calculations for double capture from He by slow multicharge ions have been carried out

  1. The electron cyclotron resonance coupled to laser ion source for charge state enhancement experiment: production of high inensity ion beams by means of hybrid ion source

    Czech Academy of Sciences Publication Activity Database

    Gammino, S.; Torrisi, L.; Ciavola, G.; Andó, L.; Celona, L.; Manciagli, S.; Krása, Josef; Láska, Leoš; Pfeifer, Miroslav; Rohlena, Karel; Mazzasalma, A. M.; Gentile, C.; Picciotto, A.; Wolowski, J.; Woryna, E.; Badziak, J.; Parys, P.; Hitz, D.; Shirkov, G. D.

    2004-01-01

    Roč. 96, č. 5 (2004), s. 2961-2967. ISSN 0021-8979 Institutional research plan: CEZ:AV0Z1010921 Keywords : laser ion sources * ECR ion sources Subject RIV: BH - Optics, Masers, Lasers Impact factor: 2.255, year: 2004

  2. Charge equilibrium processes of energetic incident ions and their range

    International Nuclear Information System (INIS)

    The charge state of energetic ions passing through a certain matter is varied by charge-exchange processes. A rate equation for charge fraction is given by using electron loss and capture cross sections in collision with a target atom under idealized condition. We solved the rate equation of the charge-exchange process of a single electron in a form of linear coupled differential equation. Our calcuiation for the range of ion were carried out for He, Ne and Ar ions passing through an atomic hydrogen gas target. We discuss the charge states of the projectile in relation to a local charge balance consituting a state of charge equilibrium in the target. (author)

  3. Radioactive decays of highly-charged ions

    Directory of Open Access Journals (Sweden)

    Gao B. S.

    2015-01-01

    Full Text Available Access to stored and cooled highly-charged radionuclides offers unprecedented opportunities to perform high-precision investigations of their decays. Since the few-electron ions, e.g. hydrogen- or helium-like ions, are quantum mechanical systems with clear electronic ground state configurations, the decay studies of such ions are performed under well-defined conditions and allow for addressing fundamental aspects of the decay process. Presented here is a compact review of the relevant experiments conducted at the Experimental Storage Ring ESR of GSI. A particular emphasis is given to the investigations of the two-body beta decay, namely the bound-state β-decay and its time-mirrored counterpart, orbital electron-capture.

  4. Importance of vacancy cascades in argon recoil-ion charge-state distributions accompanied by coincident projectile-electron capture and loss

    International Nuclear Information System (INIS)

    Argon recoil-ion charge-state distributions produced by beams of 0.7-MeV/u Cl/sup 5+,8+,10+/ have been measured by time-of-flight (TOF) techniques in coincidence with single- and double-charge-changed projectiles. In an essential improvement to the usual multinomial description of ionization in the independent-electron-ejection model, we find that inclusion of one (two) Auger vacancy cascades significantly alters the description of the recoil-ion spectra corresponding to single (double) capture. The single- and double-projectile-electron loss and capture spectra strongly resemble each other, suggesting that loss of one or two projectile electrons is closely associated with loss of one or two target L electrons, respectively. These conclusions are consistent with impact parameters inferred from determinations of mean recoil energy

  5. Preserving Charge and Oxidation State of Au(III) Ions in an Agent-Functionalized Nanocrystal Model System

    OpenAIRE

    Müllegger, Stefan; Schöfberger, Wolfgang; Rashidi, Mohammad; Lengauer, Thomas; Klappenberger, Florian; Diller, Katharina; KARA, Kamuran; Barth, Johannes V.; Rauls, Eva; Schmidt, Wolf Gero; Koch, Reinhold

    2011-01-01

    Supporting functional molecules on crystal facets is an established technique in nanotechnology. To preserve the original activity of ionic metallorganic agents on a supporting template, conservation of the charge and oxidation state of the active center is indispensable. We present a model system of a metallorganic agent that, indeed, fulfills this design criterion on a technologically relevant metal support with potential impact on Au(III)-porphyrin-functionalized nanoparticles for an impro...

  6. Simultaneous study of non equilibrated charge and excitation states of MeV/amu light atomic and molecular ions emerging from thin solid targets

    International Nuclear Information System (INIS)

    The evolution of the relative population of a given excited state of atoms H0 or ions (He+) emerging from thin carbon foils bombarded with MeV/a.m.u. atomic H0, He+ and molecular (H2+, H3+) beams has been observed in equilibrium and non-equilibrium situations which are known to occur in charge exchange processes. The comparison between charge state and photon yield (transition n = 4 - 3) variations for He+ gives new informations about capture and excitation processes in the target. Strong enhancement of the relative population of the low excited state n = 2 in the He0 emerging beam is observed in non-equilibrium regime for H0 incident beam as for hydrogen molecular incident beams. In addition, specific molecular effects occur in the equilibrium regime

  7. HICS - Highly charged ion collisions with surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Haake, Christian; Peters, Thorsten; Hopster, Johannes; Wucher, Andreas; Schleberger, Marika [Universitaet Duisburg-Essen, Fachbereich Physik, 47057 Duisburg (Germany)

    2009-07-01

    A new ion beam installation with the name HICS (highly charged ions collisions with surfaces) has been constructed to investigate the mechanisms of energy dissipation in a substrate after the impact of highly charged ions. The set-up offers high charge states (up to Ar{sup 16+} or Xe{sup 44+}) and adjustable kinetic energies which can be less than 100 eV/q. These low energies are achieved by a deceleration system which uses a device we call an ion escalator. An evaporation chamber for sample preparation is mounted and a load lock system offers in situ transport to other vacuum systems. To analyse the irradiation effects a time-of-flight system for secondary and neutral mass spectrometry (SIMS/SNMS) is installed. Inner Electronic excitations can be detected with metal-insulator-metal junctions. These detectors offer the possibility to study excitations below the work function which limits the external emission of electrons. First data measured with Ag-AlO{sub x}-Al detectors will be presented.

  8. Charge breeding simulations for radioactive ion beam production

    International Nuclear Information System (INIS)

    The charge breeding technique is used for radioactive ion beam (RIB) production in order of optimizing the re-acceleration of the radioactive element ions produced by a primary beam in a thick target. Charge breeding is achieved by means of a device capable of increasing the ion charge state from 1+ to a desired value n+. In order to get high intensity RIB, experiments with charge breeding of very high efficiency could be required. To reach this goal, the charge breeding simulation could help to optimize the high charge state production efficiency by finding more proper parameters for the radioactive 1+ ions. In this paper a device based on an electron beam ion source (EBIS) is considered. In order to study that problem, a code already developed for studying the ion selective containment in an EBIS with RF quadrupoles, BRICTEST, has been modified to simulate the ion charge state breeding rate for different 1+ ion injection conditions. Particularly, the charge breeding simulations for an EBIS with a hollow electron beam have been studied.

  9. Equilibrium and non-equilibrium charge-state distributions of 2 MeV/u sulfur ions passing through carbon foils

    Energy Technology Data Exchange (ETDEWEB)

    Imai, M. [Department of Nuclear Engineering, Kyoto University, Sakyo, Kyoto 606-8501 (Japan)], E-mail: imai@nucleng.kyoto-u.ac.jp; Sataka, M. [Nuclear Science and Engineering Directorate, Japan Atomic Energy Agency (JAEA), Tokai, Ibaraki 319-1195 (Japan); Kawatsura, K.; Takahiro, K. [Department of Chemistry and Materials Technology, Kyoto Institute of Technology, Sakyo, Kyoto 606-8585 (Japan); Komaki, K. [National Center for University Entrance Examinations, Meguro, Tokyo 153-8501 (Japan); Shibata, H. [Department of Nuclear Engineering, Kyoto University, Sakyo, Kyoto 606-8501 (Japan); Sugai, H.; Nishio, K. [Nuclear Science and Engineering Directorate, Japan Atomic Energy Agency (JAEA), Tokai, Ibaraki 319-1195 (Japan)

    2009-08-15

    Both equilibrium and non-equilibrium charge-state distributions for 2.0 MeV/u sulfur ions after passing through carbon foils were studied experimentally. For the equilibrium charge-state distribution, incident ions of S{sup 7+}, S{sup 12+}, S{sup 14+} and S{sup 16+} were injected into carbon foils 54, 98, 150 and 200 {mu}g/cm{sup 2} in thickness, whereas for the non-equilibrium distributions, new measurements for S{sup 15+} and S{sup 16+} incidences were made through carbon foils of 0.9-10 {mu}g/cm{sup 2} to supplement our previous experiments regarding S{sup 6+}-S{sup 14+} incidences [M. Imai, M. Sataka, K. Kawatsura, K. Takahiro, K. Komaki, H. Shibata, H. Sugai, K. Nishio, Nucl. Instr. and Meth. B 230 (2005) 63; M. Imai, M. Sataka, K. Kawatsura, K. Takahiro, K. Komaki, H. Shibata, H. Sugai, K. Nishio, Nucl. Instr. and Meth. B 256 (2007) 11]. Mean charge states for S{sup 6+}-S{sup 14+} incidences as functions of the penetration thickness merged at 6.9 {mu}g/cm{sup 2} and changed together until reaching equilibrium at around 100 {mu}g/cm{sup 2}, while those for S{sup 15+} and S{sup 16+} incidences took different paths to equilibrium, which was also the case for distribution widths for S{sup 6+}-S{sup 14+}, S{sup 15+} and S{sup 16+} incidences. An equilibrium mean charge state of 12.68 and distribution width of 1.11 were attained with equilibrium charge distributions between 6+ and 16+.

  10. The Solar Connection of Enhanced Heavy Ion Charge States in the Interplanetary Medium: Implications for the Flux-Rope Structure of CMEs

    Science.gov (United States)

    Gopalswamy, N.; Mäkelä, P.; Akiyama, S.; Xie, H.; Yashiro, S.; Reinard, A. A.

    2013-05-01

    We investigated a set of 54 interplanetary coronal mass ejection (ICME) events whose solar sources are very close to the disk center (within ± 15∘ from the central meridian). The ICMEs consisted of 23 magnetic-cloud (MC) events and 31 non-MC events. Our analyses suggest that the MC and non-MC ICMEs have more or less the same eruption characteristics at the Sun in terms of soft X-ray flares and CMEs. Both types have significant enhancements in ion charge states, although the non-MC structures have slightly lower levels of enhancement. The overall duration of charge-state enhancement is also considerably smaller than that in MCs as derived from solar wind plasma and magnetic signatures. We find very good correlation between the Fe and O charge-state measurements and the flare properties such as soft X-ray flare intensity and flare temperature for both MCs and non-MCs. These observations suggest that both MC and non-MC ICMEs are likely to have a flux-rope structure and the unfavorable observational geometry may be responsible for the appearance of non-MC structures at 1 AU. We do not find any evidence for an active region expansion resulting in ICMEs lacking a flux-rope structure because the mechanism of producing high charge states and the flux-rope structure at the Sun is the same for MC and non-MC events.

  11. Lifetime Measurements of Highly Charged Ions

    Energy Technology Data Exchange (ETDEWEB)

    Traebert, E. [Ruhr-Univ. Bochum (Germany). Experimentalphysik III

    2002-08-01

    How long does an atom 'live' in an excited state, when due to conservation rules and symmetry principles the 'normal' electric dipole decay to the ground state is forbidden? Then spin-changing 'intercombination' transitions and electric dipole 'forbidden' decays occur that are important for the diagnostics of low-density solar corona] and terrestrial plasmas. Regular 'allowed' and intercombination transitions in highly charged ions (picosecond and nanosecond lifetime range) have previously been measured with straight, foil-excited, fast ion beams. For ions with only one or two electrons in the valence shell, very long sections of the isoelectronic sequence have been covered this way, yielding experimental tests of theoretical predictions of transition rates that are good to a few percent. Recently the situation has become much better than this for lifetimes in the millisecond range. Here the technique of optical observation at a heavy-ion storage ring permits atomic lifetime measurements on intercombination and forbidden transitions with a precision that often is better than 1 %, which is clearly surpassing the precision range of typical conventional ion trap data. The electron beam ion trap (EBIT) exhibits a similar precision in the 'X-ray' range, and it has reached uncertainties of a few percent in some measurements of optical transitions.

  12. Lifetime Measurements of Highly Charged Ions

    International Nuclear Information System (INIS)

    How long does an atom 'live' in an excited state, when due to conservation rules and symmetry principles the 'normal' electric dipole decay to the ground state is forbidden? Then spin-changing 'intercombination' transitions and electric dipole 'forbidden' decays occur that are important for the diagnostics of low-density solar corona] and terrestrial plasmas. Regular 'allowed' and intercombination transitions in highly charged ions (picosecond and nanosecond lifetime range) have previously been measured with straight, foil-excited, fast ion beams. For ions with only one or two electrons in the valence shell, very long sections of the isoelectronic sequence have been covered this way, yielding experimental tests of theoretical predictions of transition rates that are good to a few percent. Recently the situation has become much better than this for lifetimes in the millisecond range. Here the technique of optical observation at a heavy-ion storage ring permits atomic lifetime measurements on intercombination and forbidden transitions with a precision that often is better than 1 %, which is clearly surpassing the precision range of typical conventional ion trap data. The electron beam ion trap (EBIT) exhibits a similar precision in the 'X-ray' range, and it has reached uncertainties of a few percent in some measurements of optical transitions

  13. Production of highly charged argon ions from a room temperature electron beam ion trap

    Institute of Scientific and Technical Information of China (English)

    WANG Tie-Shan; PENG Hai-Bo; Ovsyannikov V P; Kentsch U; Ullmann F; CHENG Rui; Zschornack G

    2008-01-01

    In this work.highly charged ions have been extracted from the advanced Electron Beam Ion Source (EBIS-A) developed in a scientific cooperation between the Dresden University of Technology and the DREEBIT GmbH Dresden.The charge state distributions of ions extracted from the EBIS-A are measured in and extracted in the leaky mode.3×105 Ar18+ ions per pulse are extracted in the pulse mode.The ion charge state distribution is a function of the ionization time.

  14. Strong-field Relativistic Processes in Highly Charged Ions

    OpenAIRE

    Postavaru, Octavian

    2010-01-01

    In this thesis we investigate strong-field relativistic processes in highly charged ions. In the first part,we study resonance fluorescence of laser-driven highly charged ions in the relativistic regime by solving the time-dependent master equation in a multi-level model. Our ab initio approach based on the Dirac equation allows for investigating highly relativistic ions, and, consequently, provides a sensitive means to test correlated relativistic dynamics, bound-state quantum electrodynamic...

  15. Intercombination lines in highly charged ions

    International Nuclear Information System (INIS)

    Experimental decay rates for the spin-forbidden ns2npk-1-nsnpk transitions in highly ionized Be-like, B-like, Mg-like and Al-like ions have been obtained by the beam-foil technique. Results are reported for Be-like and B-like Fe22+, Al-like Kr23+, Y26+ and Rh32+ and Mg-like Ni16+, Kr24+, Y27+ Zr28+, Nb29+ and Rh33+. For all ions in the Mg- and Al-like sequences the experimental oscillator strengths are larger than the theoretical predictions and, furthermore, the discrepancy tends to increase with increasing charge state. For both the Be- and B-like ions good agreement is found between theory and experiment. The experimental data presented here was obtained using the RILAC accelerator at RIKEN. (orig.)

  16. Magnetic hyperfine structure of the ground-state doublet in highly charged ions $^{229}$Th$^{89+,87+}$ and the Bohr-Weisskopf effect

    CERN Document Server

    Tkalya, E V

    2016-01-01

    The magnetic hyperfine (MHF) structure of the $5/2^+$(0.0 eV) ground state and the low-lying $3/2^+$(7.8 eV) isomeric state of the $^{229}$Th nucleus in highly charged ions Th$^{89+}$ and Th$^{87+}$ is calculated. The distribution of the nuclear magnetization (the Bohr-Weisskopf effect) is accounted for in the framework of the collective nuclear model with the wave functions of the Nilsson model for the unpaired neutron. The deviations of the MHF structure for the ground and isomeric states from their values in the model of point-like nuclear magnetic dipole are calculated. The influence of the mixing of the states with the same quantum number $F$ on the energy of sublevels is studied. Taking into account the mixing of states, the probabilities of the transitions between the components of MHF structure are found.

  17. Relevant effects of localized atomic interactions and surface density of states on charge transfer in ion-surface collisions

    Energy Technology Data Exchange (ETDEWEB)

    Bonetto, F.; Romero, M.A.; Garcia, E.A.; Vidal, R.; Ferron, J.; Goldberg, E.C. [Instituto de Desarrollo Tecnologico para la Industria Quimica, Consejo Nacional de Investigaciones Cientificas y Tecnicas (CONICET), Santa Fe (Argentina); Ferron, J.; Goldberg, E.C. [Universidad Nacional del Litoral, J., Dept. de Ingenieria de Materiales, Facultad de Ingenieria Quimica, Santa Fe (Argentina)

    2007-12-15

    Through a time-dependent quantum-mechanical calculation of the H{sup +} scattering by a highly oriented pyrolytic graphite (HOPG) surface, we are able to satisfactorily reproduce the interesting features we observed in ion scattering experiments in H{sup +}/HOPG system. We found that the combined effects of the semimetal character of HOPG together with the localized nature of the carbon atom states primarily determine the angular dependence and the magnitude of the ion fractions for large outgoing angles. The spin fluctuation effects (not considered in the present calculation) are discussed as one of the the main causes of the disagreement between the spinless theory results and the experiments for small exit angles. (authors)

  18. Holographic heavy ion collisions with baryon charge

    CERN Document Server

    Casalderrey-Solana, Jorge; van der Schee, Wilke; Triana, Miquel

    2016-01-01

    We numerically simulate collisions of charged shockwaves in Einstein-Maxwell theory in anti-de Sitter space as a toy model of heavy ion collisions with non-zero baryon charge. The stress tensor and the baryon current become well described by charged hydrodynamics at roughly the same time. The effect of the charge density on generic observables is typically no larger than 15\\%. %The rapidity profile of the charge is wider than the profile of the local energy density. We find significant stopping of the baryon charge and compare our results with those in heavy ion collision experiments.

  19. Magnetic hyperfine structure of the ground-state doublet in highly charged ions 89+,87+229Th and the Bohr-Weisskopf effect

    Science.gov (United States)

    Tkalya, E. V.; Nikolaev, A. V.

    2016-07-01

    Background: The search for new opportunities to investigate the low-energy level in the 229Th nucleus, which is nowadays intensively studied experimentally, has motivated us to theoretical studies of the magnetic hyperfine (MHF) structure of the 5 /2+ (0.0 eV) ground state and the low-lying 3 /2+ (7.8 eV) isomeric state in highly charged 89+229Th and 87+229Th ions. Purpose: The aim is to calculate, with the maximal precision presently achievable, the energy of levels of the hyperfine structure of the 229Th ground-state doublet in highly charged ions and the probability of radiative transitions between these levels. Methods: The distribution of the nuclear magnetization (the Bohr-Weisskopf effect) is accounted for in the framework of the collective nuclear model with Nilsson model wave functions for the unpaired neutron. Numerical calculations using precise atomic density functional theory methods, with full account of the electron self-consistent field, have been performed for the electron structure inside and outside the nuclear region. Results: The deviations of the MHF structure for the ground and isomeric states from their values in a model of a pointlike nuclear magnetic dipole are calculated. The influence of the mixing of the states with the same quantum number F on the energy of sublevels is studied. Taking into account the mixing of states, the probabilities of the transitions between the components of the MHF structure are calculated. Conclusions: Our findings are relevant for experiments with highly ionized 229Th ions in a storage ring at an accelerator facility.

  20. Photons shedding light on electron capture by highly charged ions

    OpenAIRE

    Hoekstra, Romke Anne

    1990-01-01

    In this thesis charge transfer is studied in collisions of highly charged ions (Aq+) with neutral particles (B). Because the electron is captured resonantly (i.e. without its binding energy) by the ion, a limited number of highly excited states (characterized by the quantum numbers nlm) is preferentially populated. In the experimental work described in this thesis we have measured state selective electron capture cross sections by means of Photon Emission Spectroscopy. Especially, the most fu...

  1. Computation of Ion Charge State Distributions After Inner-shell Ionization in Ne, Ar and Kr Atoms Using Monte Carlo Simulation

    International Nuclear Information System (INIS)

    Atomic reorganization starts by filling the initially inner-shell vacancy by a radiative transition (x-ray) or by a non-radiative transition (Auger and Coster-Kronig processes). New vacancies created during this atomic reorganization may in turn be filled by further radiative and non-radiative transitions until all vacancies reach the outermost occupied shells. The production of inner-shell vacancy in an atom and the de-excitation decays through radiative and non-radiative transitions may result in a change of the atomic potential; this change leads to the emission of an additional electron in the continuum (electron shake-off processes). In the present work, the ion charge state distributions (CSD) and mean atomic charge ions produced from inner shell vacancy de-excitation decay are calculated for neutral Ne , Ar and Kr atoms. The calculations are carried out using Monte Carlo (MC) technique to simulate the cascade development after primary vacancy production. The radiative and non-radiative transitions for each vacancy are calculated in the simulation. In addition, the change of transition energies and transition rates due to multi vacancies produced in the atomic configurations through the cascade development are considered in the present work. It is found that considering the electron shake off process and closing of non-allowed non-radiative channels improves the results of both charge state distributions (CSD) and average charge state. To check the validity of the present calculations, the results obtained are compared with available theoretical and experimental data. The present results are found to agree well with the available theoretical and experimental values. (author)

  2. Computation of Ion Charge State Distributions After Inner-Shell Ionization In Ne, Ar And Kr Atoms Using Monte Carlo Simulation

    International Nuclear Information System (INIS)

    Atomic reorganization starts by filling the initially inner-shell vacancy by a radiative transition (x-ray) or by a non-radiative transition (Auger and Coster-Kronig processes). New vacancies created during this atomic reorganization may in turn be filled by further radiative and non-radiative transitions until all vacancies reach the outermost occupied shells. The production of inner-shell vacancy in an atom and the de-excitation decays through radiative and non-radiative transitions may result in a change of the atomic potential; this change leads to the emission of an additional electron in the continuum (electron shake-off processes). In the present work, the ion charge state distributions (CSD) and mean atomic charge ions produced from inner-shell vacancy de-excitation decay are calculated for neutral Ne, Ar and Kr atoms. The calculations are carried out using Monte Carlo (MC) technique to simulate the cascade development after primary vacancy production. The radiative and non-radiative transitions for each vacancy are calculated in the simulation. In addition, the change of transition energies and transition rates due to multi vacancies produced in the atomic configurations through the cascade development are considered in the present work. It is found that considering the electron shake--off process and closing of non-allowed non-radiative channels improves the results of both charge state distributions (CSD) and average charge state. To check the validity of the present calculations, the results obtained are compared with available theoretical and experimental data. The present results are found to agree well with the available theoretical and experimental values.

  3. Precision mass measurements of highly charged ions

    Science.gov (United States)

    Kwiatkowski, A. A.; Bale, J. C.; Brunner, T.; Chaudhuri, A.; Chowdhury, U.; Ettenauer, S.; Frekers, D.; Gallant, A. T.; Grossheim, A.; Lennarz, A.; Mane, E.; MacDonald, T. D.; Schultz, B. E.; Simon, M. C.; Simon, V. V.; Dilling, J.

    2012-10-01

    The reputation of Penning trap mass spectrometry for accuracy and precision was established with singly charged ions (SCI); however, the achievable precision and resolving power can be extended by using highly charged ions (HCI). The TITAN facility has demonstrated these enhancements for long-lived (T1/2>=50 ms) isobars and low-lying isomers, including ^71Ge^21+, ^74Rb^8+, ^78Rb^8+, and ^98Rb^15+. The Q-value of ^71Ge enters into the neutrino cross section, and the use of HCI reduced the resolving power required to distinguish the isobars from 3 x 10^5 to 20. The precision achieved in the measurement of ^74Rb^8+, a superallowed β-emitter and candidate to test the CVC hypothesis, rivaled earlier measurements with SCI in a fraction of the time. The 111.19(22) keV isomeric state in ^78Rb was resolved from the ground state. Mass measurements of neutron-rich Rb and Sr isotopes near A = 100 aid in determining the r-process pathway. Advanced ion manipulation techniques and recent results will be presented.

  4. Heavy Coronal Ions in the Heliosphere: I. Global Distribution of Charge-states of C, N, O, Mg, Si and S

    OpenAIRE

    Grzedzielski, S.; Wachowicz, M. E.; Bzowski, M.; Izmodenov, V.

    2008-01-01

    Aims: Investigate/Study de-charging of solar wind C, N, O, Mg, Si and S ions and assess fluxes of resulting ENA in the heliosphere. Methods: The model treats the heavy ions as test particles convected by (and in a particular case also diffusing through) a hydrodynamically calculated background plasma flow, from 1 AU to the termination shock (TS), to heliosheath (HS) and finally to heliospheric tail (HT). The ions undergo radiative and dielectronic recombinations, charge exchanges, photo- and ...

  5. Electron configuration and charge state of electrically active Cu, Ag and Au ions in ZnSe

    International Nuclear Information System (INIS)

    The Hall effect, electrical conductivity and electron mobility are investigated at temperatures between 55 and 500 K in n-ZnSe crystals doped with Cu, Ag or Au. The presence of a small amount of Cu atoms leads to an inversion of the sign of the Hall coefficient at temperatures above 300 K. Anomalous temperature dependence of the electron mobility is observed in the samples with low Cu concentration (Zn+ (d10) and CuZn2+ (d9), and two acceptor levels near the valence band. Silver and gold exist in single-charged states AgZn+ and AuZn+ with d10 electron configuration forming single energy levels near the valence band. Au atoms form mainly interstitial Aui donors at low doping concentrations and substitutional AuZn and AuZn-based acceptors at high doping concentrations. Time stimulation of the amphoteric properties of Ag is discussed

  6. A novel method for state of charge estimation of lithium-ion batteries using a nonlinear observer

    Science.gov (United States)

    Xia, Bizhong; Chen, Chaoren; Tian, Yong; Sun, Wei; Xu, Zhihui; Zheng, Weiwei

    2014-12-01

    The state of charge (SOC) is important for the safety and reliability of battery operation since it indicates the remaining capacity of a battery. However, as the internal state of each cell cannot be directly measured, the value of the SOC has to be estimated. In this paper, a novel method for SOC estimation in electric vehicles (EVs) using a nonlinear observer (NLO) is presented. One advantage of this method is that it does not need complicated matrix operations, so the computation cost can be reduced. As a key step in design of the nonlinear observer, the state-space equations based on the equivalent circuit model are derived. The Lyapunov stability theory is employed to prove the convergence of the nonlinear observer. Four experiments are carried out to evaluate the performance of the presented method. The results show that the SOC estimation error converges to 3% within 130 s while the initial SOC error reaches 20%, and does not exceed 4.5% while the measurement suffers both 2.5% voltage noise and 5% current noise. Besides, the presented method has advantages over the extended Kalman filter (EKF) and sliding mode observer (SMO) algorithms in terms of computation cost, estimation accuracy and convergence rate.

  7. Experimental Evidence for Space-Charge Effects between Ions of the Same Mass-to-Charge in Fourier-Transform Ion Cyclotron Resonance Mass Spectrometry

    OpenAIRE

    Wong, Richard L.; Amster, I. Jonathan

    2007-01-01

    It is often stated that ions of the same mass-to-charge do not induce space-charge frequency shifts among themselves in an ion cyclotron resonance mass spectrometry measurement. Here, we demonstrate space-charge induced frequency shifts for ions of a single mass-to-charge. The monoisotopic atomic ion, Cs+, was used for this study. The measured frequency is observed to decrease linearly with an increase in the number of ions, as has been reported previously for space-charge effects between ion...

  8. Charge exchange between hydrogen atoms and fully stripped heavy ions

    International Nuclear Information System (INIS)

    Charge exchange between multicharged ions and background atomic and molecular gases represents one of the limitations to the attainment of high charge states in heavy ion sources, particularly containment sources. An attempt is made to study systematically a particularly simple but in many respects representative class of such reactions, namely charge transfer between atomic hydrogen and fully stripped heavy ions. Approximate cross sections for these processes in the low keV range of collision energies were obtained using a multistate Landau--Zener method. The energy and Z dependences of the cross sections are discussed

  9. Cross sections for ion-molecular reactions in hydrogen systems and for charge transfer reactions of slow multiply charged ions

    International Nuclear Information System (INIS)

    Cross sections of ion-molecular reactions in hydrogen systems of H+-H2, H2+-H2 and H3+-H2 and charge transfer cross sections of multiply charged ions in atomic and molecular targets are presented in graphs and tables of the part A, B and C. All data presented for 99 collision systems have been measured systematically using an octo-pole ion beam guide (OPIG) technique till now since 1985. The part A is for ion-molecular reactions in hydrogen systems. In the lower energy region below few eV in center-of-mass systems, it is seen obviously at a glance that the ion-molecular reaction in hydrogen systems is dominated by H3+ formation process. In the energy region from few eV to few hundred eV in center-of-mass systems, many reaction channels of decay processes from intermediate molecular states seem to be opened resonantly. Some of cross section data in the part B for charge transfer reactions of low-charged ions produced by a conventional electron impact type (Nier type) ion source should be noted to strongly depend on the electron impact energy due to contamination of low lying metastable states in projectile ions. The part C is for charge transfer reactions of multiply charged ions extracted from a small type of electron beam ion source (Mini-EBIS). In measurements using the mini-EBIS, no evidence of metastable ions existing in the primary ion beam has been found except for doubly charged ion beam. The higher energy end of the present cross sections are connected with previous data in fairly good

  10. Confinement of multiply charged ions in an ECRH mirror plasma

    International Nuclear Information System (INIS)

    This thesis is an experimental study of multiply charged ions in the Constance B mirror experiment. By measuring the ion densities, end loss fluxes and ion temperatures, the parallel confinement times for the first five charge states of oxygen and neon plasmas are determined. The parallel ion confinement times increase with charge state and peak on axis, both indications of an ion-confining potential dip created by the hot electrons. The radial profile of ion end loss is usually hollow due to large ion radial transport (τparalleli ∼ τperpendiculari), with the peak fluxes occurring at the edge of the electron cyclotron resonance zone. Several attempts are made to increase the end loss of selected ion species. Using minority ICRH, the end loss flux of resonant ions increases by 20% in cases when radial transport induced by ICRH is not too severe. A large antenna voltage can also extinguish the plasma. By adding helium to an oxygen plasma, the end loss of O6+ increases by 80% due to decreased ion radial transport. An ion model is developed to predict the ion densities, end loss fluxes and confinement times in the plasma center using the ion particle balance equations, the quasineutrality condition and theoretical confinement time formulas. The model generally agrees with the experimental data for oxygen and neon plasmas to within experimental error. Under certain conditions spatial diffusion appears to determine the parallel ion confinement time of the highest charge states. For oxygen plasmas during ICRH, the measured parallel confinement time of the resonant ions is much shorter than their theoretical value, probably due to rf diffusion of the ions into the loss cone. 58 refs., 101 figs., 16 tabs

  11. The charge spectrum of positive ions in a hydrogen aurora

    Science.gov (United States)

    Lynch, J.; Pulliam, D.; Leach, R.; Scherb, F.

    1976-01-01

    An auroral ion charge spectrometer was flown into a hydrogen aurora on a Javelin sounding rocket launched from Churchill, Manitoba. The instrument contained an electrostatic analyzer which selected particles with incident energy per unit charge up to 20 keV/charge and an 80-kV power supply which accelerated these ions onto an array of solid state detectors. Ions tentatively identified as H(+), He(+2), and O(+) were detected from 225 to 820 km in altitude. The experiment did not discriminate between H(+) and He(+), or between O(+), N(+), and C(+). Upper limits of highly charged heavy ion abundances have been set at 20% of the He(+2) and 0.15% of the H(+). It is concluded that both terrestrial and solar wind sources play significant roles in auroral ion precipitation.

  12. Electron capture by highly charged ions from surfaces and gases

    Energy Technology Data Exchange (ETDEWEB)

    Allen, F.

    2008-01-11

    In this study highly charged ions produced in Electron Beam Ion Traps are used to investigate electron capture from surfaces and gases. The experiments with gas targets focus on spectroscopic measurements of the K-shell x-rays emitted at the end of radiative cascades following electron capture into Rydberg states of Ar{sup 17+} and Ar{sup 18+} ions as a function of collision energy. The ions are extracted from an Electron Beam Ion Trap at an energy of 2 keVu{sup -1}, charge-selected and then decelerated down to 5 eVu{sup -1} for interaction with an argon gas target. For decreasing collision energies a shift to electron capture into low orbital angular momentum capture states is observed. Comparative measurements of the K-shell x-ray emission following electron capture by Ar{sup 17+} and Ar{sup 18+} ions from background gas in the trap are made and a discrepancy in the results compared with those from the extraction experiments is found. Possible explanations are discussed. For the investigation of electron capture from surfaces, highly charged ions are extracted from an Electron Beam Ion Trap at energies of 2 to 3 keVu{sup -1}, charge-selected and directed onto targets comprising arrays of nanoscale apertures in silicon nitride membranes. The highly charged ions implemented are Ar{sup 16+} and Xe{sup 44+} and the aperture targets are formed by focused ion beam drilling in combination with ion beam assisted thin film deposition, achieving hole diameters of 50 to 300 nm and aspect ratios of 1:5 to 3:2. After transport through the nanoscale apertures the ions pass through an electrostatic charge state analyzer and are detected. The percentage of electron capture from the aperture walls is found to be much lower than model predictions and the results are discussed in terms of a capillary guiding mechanism. (orig.)

  13. Electron capture by highly charged ions from surfaces and gases

    International Nuclear Information System (INIS)

    In this study highly charged ions produced in Electron Beam Ion Traps are used to investigate electron capture from surfaces and gases. The experiments with gas targets focus on spectroscopic measurements of the K-shell x-rays emitted at the end of radiative cascades following electron capture into Rydberg states of Ar17+ and Ar18+ ions as a function of collision energy. The ions are extracted from an Electron Beam Ion Trap at an energy of 2 keVu-1, charge-selected and then decelerated down to 5 eVu-1 for interaction with an argon gas target. For decreasing collision energies a shift to electron capture into low orbital angular momentum capture states is observed. Comparative measurements of the K-shell x-ray emission following electron capture by Ar17+ and Ar18+ ions from background gas in the trap are made and a discrepancy in the results compared with those from the extraction experiments is found. Possible explanations are discussed. For the investigation of electron capture from surfaces, highly charged ions are extracted from an Electron Beam Ion Trap at energies of 2 to 3 keVu-1, charge-selected and directed onto targets comprising arrays of nanoscale apertures in silicon nitride membranes. The highly charged ions implemented are Ar16+ and Xe44+ and the aperture targets are formed by focused ion beam drilling in combination with ion beam assisted thin film deposition, achieving hole diameters of 50 to 300 nm and aspect ratios of 1:5 to 3:2. After transport through the nanoscale apertures the ions pass through an electrostatic charge state analyzer and are detected. The percentage of electron capture from the aperture walls is found to be much lower than model predictions and the results are discussed in terms of a capillary guiding mechanism. (orig.)

  14. Atomic physics experiments with trapped and cooled highly charged ions

    OpenAIRE

    Kluge, H.-J.; Quint, W; Winters, D. F. A

    2007-01-01

    Trapping and cooling techniques have become very important for many fundamental experiments in atomic physics. When applied to highly charged ions confined in Penning traps, these procedures are very effective for testing quantum electrodynamics in extreme electromagnetic fields produced by heavy highly charged ions such as uranium U$^{91+}$. In addition, fundamental constants or nuclear ground state properties can be determined with high accuracy in these simple systems. Finally, by studying...

  15. Charge breeding of radioactive ions with EBIS and EBIT

    CERN Document Server

    Wenander, Fredrik

    2010-01-01

    A charge state breeder, which transforms externally injected singly charged ions to a higher charge state q+, is an important tool which has applications within atomic, nuclear and even particle physics. The charge breeding concept of radioactive ions has already been demonstrated at REX-ISOLDE/CERN with the use of an Electron beam Ion Source (EBIS) and at several facilities employing Electron Resonance Cyclotron Ion Sources (ECRIS). As will be demonstrated in this paper, EBIS and Electron Beam Ion Traps (EBIT), are well suited for the task as they are capable of delivering clean, highly charged beams within a short transformation time. The increasing demand for highly charged ions of all kind of elements and isotopes, stable and radioactive, to be used for low-energy experiments such as TITAN at TRIUMF and MATS at FAIR, but also for post-acceleration to higher energies, is now pushing the development of the breeders. The next challenge will be to satisfy the needs, for example space-charge capacity, of the s...

  16. Estimation method of state-of-charge for lithium-ion battery used in hybrid electric vehicles based on variable structure extended kalman filter

    Science.gov (United States)

    Sun, Yong; Ma, Zilin; Tang, Gongyou; Chen, Zheng; Zhang, Nong

    2016-03-01

    Since the main power source of hybrid electric vehicle(HEV) is supplied by the power battery, the predicted performance of power battery, especially the state-of-charge(SOC) estimation has attracted great attention in the area of HEV. However, the value of SOC estimation could not be greatly precise so that the running performance of HEV is greatly affected. A variable structure extended kalman filter(VSEKF)-based estimation method, which could be used to analyze the SOC of lithium-ion battery in the fixed driving condition, is presented. First, the general lower-order battery equivalent circuit model(GLM), which includes column accumulation model, open circuit voltage model and the SOC output model, is established, and the off-line and online model parameters are calculated with hybrid pulse power characteristics(HPPC) test data. Next, a VSEKF estimation method of SOC, which integrates the ampere-hour(Ah) integration method and the extended Kalman filter(EKF) method, is executed with different adaptive weighting coefficients, which are determined according to the different values of open-circuit voltage obtained in the corresponding charging or discharging processes. According to the experimental analysis, the faster convergence speed and more accurate simulating results could be obtained using the VSEKF method in the running performance of HEV. The error rate of SOC estimation with the VSEKF method is focused in the range of 5% to 10% comparing with the range of 20% to 30% using the EKF method and the Ah integration method. In Summary, the accuracy of the SOC estimation in the lithium-ion battery cell and the pack of lithium-ion battery system, which is obtained utilizing the VSEKF method has been significantly improved comparing with the Ah integration method and the EKF method. The VSEKF method utilizing in the SOC estimation in the lithium-ion pack of HEV can be widely used in practical driving conditions.

  17. A modified model based state of charge estimation of power lithium-ion batteries using unscented Kalman filter

    Science.gov (United States)

    Tian, Yong; Xia, Bizhong; Sun, Wei; Xu, Zhihui; Zheng, Weiwei

    2014-12-01

    Accurate estimation for the state of charge (SOC) is one of the most important aspects of a battery management system (BMS) in electric vehicles (EVs) as it provides drivers with the EVs' remaining range. However, it is difficult to get an accurate SOC, because its value cannot be directly measured and is affected by various factors, such as the operating temperature, current rate and cycle number. In this paper, a modified equivalent circuit model is presented to include the impact of different current rates and SOCs on the battery internal resistance, and the impact of different temperatures and current rates on the battery capacity. Besides, a linear-averaging method is presented to calculate the internal resistance and practical capacity correction factors according to data collected from the experimental bench and saved as look-up tables. The unscented Kalman filter (UKF) algorithm is then introduced to estimate the SOC according to the presented model. Experiments based on actual urban driving cycles are carried out to evaluate the performance of the presented method by comparing with two existed methods. Experimental results show that the proposed method can reduce the computation cost and improve the SOC estimation accuracy simultaneously.

  18. Electron impact single ionization of multiply charged iron ions

    International Nuclear Information System (INIS)

    Employing the animated crossed-beams technique, absolute cross sections for electron impact single ionization of the iron isonuclear sequence are measured for charge states q=1-6 for electron energies from threshold up to 1 keV, as well as for the intermediate charge states q=9,10 up to an electron energy of 5 keV. The cross sections observed for Feq+ ions in charge states q=1-4, 9 and 10 show a significant ionization signal below the respective ground state threshold resulting from ions in excited, long-lived metastable states in the parent ion beam. In the case of Fe5+ and Fe6+ no metastable components are found. The experimental results are in good agreement with the theoretical predictions if excitation-autoionization processes are taken into account. Our measured cross sections are also in good agreement with experimental results of other groups. (author)

  19. A New Technique for Diagnosing Multi-charged Ion Beams Produced by ECR Ion Source

    Institute of Scientific and Technical Information of China (English)

    ZhangZimin; ZhaoHongwei; CaoYun; MaLei; MaBaohua; LiJinyu; WangHui; FengYucheng; DuJunfeng

    2003-01-01

    In order to study the transmission properties of multi-charged ion beams between the ECR ion source and the analyzing magnet, a new diagnostic system composed of three Wien-filters with three single-wires has been built and installed on the IMP ECR source test bcnch. The single-wire is used to measure the beam profile and the beam density distribution, and the Wien-filter is used to measure the charge state distribution of ion beam.

  20. Handbook for highly charged ion spectroscopic research

    CERN Document Server

    Hutton, Roger; Currell, Fred; Martinson, Indrek; Hagmann, Siegbert

    2011-01-01

    Highly charged ions are key research objects in atomic physics. Precision spectroscopy of such ions provides a powerful tool for exploring relativistic and quantum electrodynamics effects. Additionally, the interaction of high-energy heavy-ions with matter is itself a topic of importance in many areas of applied physics, including fusion and plasma physics, accelerator physics, materials science and semiconductor device preparation and behavior. This work provides a complete overview of modern methods of studying highly charged ions. With chapters covering everything from the essential backgro

  1. Highly charged ion beam applied to lithography technique.

    Science.gov (United States)

    Momota, Sadao; Nojiri, Yoichi; Taniguchi, Jun; Miyamoto, Iwao; Morita, Noboru; Kawasegi, Noritaka

    2008-02-01

    In various fields of nanotechnology, the importance of nanoscale three-dimensional (3D) structures is increasing. In order to develop an efficient process to fabricate nanoscale 3D structures, we have applied highly charged ion (HCI) beams to the ion-beam lithography (IBL) technique. Ar-ion beams with various charge states (1+ to 9+) were applied to fabricate spin on glass (SOG) and Si by means of the IBL technique. The Ar ions were prepared by a facility built at Kochi University of Technology, which includes an electron cyclotron resonance ion source (NANOGAN, 10 GHz). IBL fabrication was performed as a function of not only the charge state but also the energy and the dose of Ar ions. The present results show that the application of an Ar(9+) beam reduces the etching time for SOG and enhances the etching depth compared with those observed with Ar ions in lower charged states. Considering the high-energy deposition of HCI at a surface, the former phenomena can be understood consistently. Also, the latter phenomena can be understood based on anomalously deep structural changes, which are remarkable for glasses. Furthermore, it has also been shown that the etching depth can be easily controlled with the kinetic energy of the Ar ions. These results show the possibilities of the IBL technique with HCI beams in the field of nanoscale 3D fabrication. PMID:18315242

  2. Multiply charged ion beams from solid substances

    International Nuclear Information System (INIS)

    The mVINIS Ion Source has enabled us to obtain multiply charged ion beams from gases as well as from solid materials. The solid substance ion beams were produced by using two techniques: a) the evaporation of metals by using the inlet system based on mini-oven and b) the metal-ions-from volatile-compounds method (MIVOC) by using the modified gas inlet system. In the production of high current stable ion beams of solids with relatively high melting points (over 1000 deg) were made great efforts. The B3+ ion beam current of over 300 μA is one of the most intensive beams extracted until now. The obtained multiply charged ion beam spectra of solid substances (B, Fe and Zn) are presented as well as some of the corresponding experimental results achieved during the modification of polymers, carbon materials and fullerenes. (author)

  3. Atomic collisions in fusion plasmas involving multiply charged ions

    International Nuclear Information System (INIS)

    A short survey is given on atomic collisions involving multiply charged ions. The basic features of charge transfer processes in ion-ion and ion-atom collisions relevant to fusion plasmas are discussed. (author)

  4. Single and multiple photoionization of Wq+ tungsten ions in charge states q=1,2,..,5: experiment and theory

    International Nuclear Information System (INIS)

    Absolute cross sections for single and multiple photoionization of Wq+ ions have been measured in a photon-ion merged beam setup employing synchrotron radiation from the Advanced Light Source. The experimental data are compared to large-scale close-coupling calculations within the Dirac-Coulomb R-matrix (DARC) approximation.

  5. Measurements of aerosol charging states in Helsinki, Finland

    Directory of Open Access Journals (Sweden)

    S. Gagné

    2011-05-01

    Full Text Available The charging state of aerosol populations was measured with an Ion-DMPS in Helsinki, Finland between December 2008 and February 2010. Based on the charging states, we calculated the ion-induced nucleation fraction to be around 0.8 % ± 0.9 %. We review the role of ion-induced nucleation and propose different explanations for a low ion-induced nucleation participation in urban areas. We present a new method to retrieve the average charging state for an event, and a given size. We also use a new theoretical framework that allows for different concentrations of small cluster ions for different polarities (polarity asymmetry. We extrapolate the ion-induced fraction using polarity symmetry and asymmetry. Finally, a method to calculate the growth rates from the variation of the charging state as a function of the particle diameter using polarity symmetry and asymmetry is presented and used on a selection of new particle formation events.

  6. Production of High-Intensity, Highly Charged Ions

    CERN Document Server

    Gammino, S

    2013-01-01

    In the past three decades, the development of nuclear physics facilities for fundamental and applied science purposes has required an increasing current of multicharged ion beams. Multiple ionization implies the formation of dense and energetic plasmas, which, in turn, requires specific plasma trapping configurations. Two types of ion source have been able to produce very high charge states in a reliable and reproducible way: electron beam ion sources (EBIS) and electron cyclotron resonance ion sources (ECRIS). Multiple ionization is also obtained in laser-generated plasmas (laser ion sources (LIS)), where the high-energy electrons and the extremely high electron density allow step-by-step ionization, but the reproducibility is poor. This chapter discusses the atomic physics background at the basis of the production of highly charged ions and describes the scientific and technological features of the most advanced ion sources. Particular attention is paid to ECRIS and the latest developments, since they now r...

  7. Final state effects on charge asymmetry of pion elliptic flow in high-energy heavy-ion collisions

    CERN Document Server

    Ma, Guo-Liang

    2014-01-01

    Within a multi-phase transport (AMPT) model with string melting mechanism and an imported electric charge quadrupole distribution in the initial partonic coordinate space, the elliptic flow asymmetry between positive and negative pions is investigated. The slope parameter $r$ of the linear dependence of $\\Delta v_{2}=v_{2}(\\pi^{-})-v_{2}(\\pi^{+})$ on $A_{ch}=(N^{+}-N^{-})/(N^{+}+N^{-})$ is yielded by the conversion from an initial electric charge quadrupole distribution to a charge-dependent elliptic flow via a strong parton cascade process. The slope parameter $r$ is increased by the hadronization of coalescence, and then decreased by final resonance decays. Because the slope parameter $r$ is very sensitive to both initial electric charge quadrupole percentage and centrality, a helpful constraint of the effect from chiral magnetic wave is extracted out in Au+Au collisions at the top RHIC energy.

  8. Comparison of Nonlinear Filtering Methods for Estimating the State of Charge of Li4Ti5O12 Lithium-Ion Battery

    Directory of Open Access Journals (Sweden)

    Jianping Gao

    2015-01-01

    Full Text Available Accurate state of charge (SoC estimation is of great significance for the lithium-ion battery to ensure its safety operation and to prevent it from overcharging or overdischarging. To achieve reliable SoC estimation for Li4Ti5O12 lithium-ion battery cell, three filtering methods have been compared and evaluated. A main contribution of this study is that a general three-step model-based battery SoC estimation scheme has been proposed. It includes the processes of battery data measurement, parametric modeling, and model-based SoC estimation. With the proposed general scheme, multiple types of model-based SoC estimators have been developed and evaluated for battery management system application. The detailed comparisons on three advanced adaptive filter techniques, which include extend Kalman filter, unscented Kalman filter, and adaptive extend Kalman filter (AEKF, have been implemented with a Li4Ti5O12 lithium-ion battery. The experimental results indicate that the proposed model-based SoC estimation approach with AEKF algorithm, which uses the covariance matching technique, performs well with good accuracy and robustness; the mean absolute error of the SoC estimation is within 1% especially with big SoC initial error.

  9. Production of High-Intensity, Highly Charged Ions

    OpenAIRE

    S. GamminoINFN, LNS, Catania

    2015-01-01

    In the past three decades, the development of nuclear physics facilities for fundamental and applied science purposes has required an increasing current of multicharged ion beams. Multiple ionization implies the formation of dense and energetic plasmas, which, in turn, requires specific plasma trapping configurations. Two types of ion source have been able to produce very high charge states in a reliable and reproducible way: electron beam ion sources (EBIS) and electron cyclotron resonance i...

  10. Online model-based estimation of state-of-charge and open-circuit voltage of lithium-ion batteries in electric vehicles

    International Nuclear Information System (INIS)

    This paper presents a method to estimate the state-of-charge (SOC) of a lithium-ion battery, based on an online identification of its open-circuit voltage (OCV), according to the battery’s intrinsic relationship between the SOC and the OCV for application in electric vehicles. Firstly an equivalent circuit model with n RC networks is employed modeling the polarization characteristic and the dynamic behavior of the lithium-ion battery, the corresponding equations are built to describe its electric behavior and a recursive function is deduced for the online identification of the OCV, which is implemented by a recursive least squares (RLS) algorithm with an optimal forgetting factor. The models with different RC networks are evaluated based on the terminal voltage comparisons between the model-based simulation and the experiment. Then the OCV-SOC lookup table is built based on the experimental data performed by a linear interpolation of the battery voltages at the same SOC during two consecutive discharge and charge cycles. Finally a verifying experiment is carried out based on nine Urban Dynamometer Driving Schedules. It indicates that the proposed method can ensure an acceptable accuracy of SOC estimation for online application with a maximum error being less than 5.0%. -- Highlights: ► An equivalent circuit model with n RC networks is built for lithium-ion batteries. ► A recursive function is deduced for the online estimation of the model parameters like OCV and RO. ► The relationship between SOC and OCV is built with a linear interpolation method by experiments. ► The experiments show the online model-based SOC estimation is reasonable with enough accuracy.

  11. Atomic physics experiments with trapped and cooled highly charged ions

    CERN Document Server

    Kluge, H -J; Winters, D F A

    2007-01-01

    Trapping and cooling techniques have become very important for many fundamental experiments in atomic physics. When applied to highly charged ions confined in Penning traps, these procedures are very effective for testing quantum electrodynamics in extreme electromagnetic fields produced by heavy highly charged ions such as uranium U$^{91+}$. In addition, fundamental constants or nuclear ground state properties can be determined with high accuracy in these simple systems. Finally, by studying a single trapped radioactive ion, its nuclear decay can be studied in detail by observing the disappearance of the signal of the mother and the appearance of that of the daughter isotope. Such experiments on highly charged ions at extremely low energy will become possible by the HITRAP facility which is currently being built up at GSI. Also the future Facility for Antiproton and Ion Research (FAIR) will be briefly described which is expected to be operational by 2014.

  12. Comparisons of Modeling and State of Charge Estimation for Lithium-Ion Battery Based on Fractional Order and Integral Order Methods

    Directory of Open Access Journals (Sweden)

    Renxin Xiao

    2016-03-01

    Full Text Available In order to properly manage lithium-ion batteries of electric vehicles (EVs, it is essential to build the battery model and estimate the state of charge (SOC. In this paper, the fractional order forms of Thevenin and partnership for a new generation of vehicles (PNGV models are built, of which the model parameters including the fractional orders and the corresponding resistance and capacitance values are simultaneously identified based on genetic algorithm (GA. The relationships between different model parameters and SOC are established and analyzed. The calculation precisions of the fractional order model (FOM and integral order model (IOM are validated and compared under hybrid test cycles. Finally, extended Kalman filter (EKF is employed to estimate the SOC based on different models. The results prove that the FOMs can simulate the output voltage more accurately and the fractional order EKF (FOEKF can estimate the SOC more precisely under dynamic conditions.

  13. Spectroscopy with trapped highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Beiersdorfer, P

    2008-01-23

    We give an overview of atomic spectroscopy performed on electron beam ion traps at various locations throughout the world. Spectroscopy at these facilities contributes to various areas of science and engineering, including but not limited to basic atomic physics, astrophysics, extreme ultraviolet lithography, and the development of density and temperature diagnostics of fusion plasmas. These contributions are accomplished by generating, for example, spectral surveys, making precise radiative lifetime measurements, accounting for radiative power emitted in a given wavelength band, illucidating isotopic effects, and testing collisional-radiative models. While spectroscopy with electron beam ion traps had originally focused on the x-ray emission from highly charged ions interacting with the electron beam, the operating modes of such devices have expanded to study radiation in almost all wavelength bands from the visible to the hard x-ray region; and at several facilities the ions can be studied even in the absence of an electron beam. Photon emission after charge exchange or laser excitation has been observed, and the work is no longer restricted to highly charged ions. Much of the experimental capabilities are unique to electron beam ion traps, and the work performed with these devices cannot be undertaken elsewhere. However, in other areas the work on electron beam ion traps rivals the spectroscopy performed with conventional ion traps or heavy-ion storage rings. The examples we present highlight many of the capabilities of the existing electron beam ion traps and their contributions to physics.

  14. Evaluation of Lithium-Ion Battery Equivalent Circuit Models for State of Charge Estimation by an Experimental Approach

    OpenAIRE

    Jinxin Fan; Hongwen He; Rui Xiong

    2011-01-01

    To improve the use of lithium-ion batteries in electric vehicle (EV) applications, evaluations and comparisons of different equivalent circuit models are presented in this paper. Based on an analysis of the traditional lithium-ion battery equivalent circuit models such as the Rint, RC, Thevenin and PNGV models, an improved Thevenin model, named dual polarization (DP) model, is put forward by adding an extra RC to simulate the electrochemical polarization and concentration polarization separat...

  15. Ionic charge state measurements in solar energetic particle events

    International Nuclear Information System (INIS)

    With the launch of the Advanced Composition Explorer, it has become possible through the SEPICA instrument to make direct ionic charge state measurements for individual Solar Energetic Particle events. In large events, the charge state may even be measured as a function of time, revealing changes that may be created by phenomena such as injections from different acceleration mechanisms, or confinement by magnetic field structures. The charge state can be a sensitive indicator of separate SEP populations. Several examples of SEP events will be presented. One of these, the November, 1997 event, displayed a trend in which the mean charge state for several ions increased with energy. These measurements may be the result of several processes, including a mixture of plasma with different source and acceleration histories, and abundance formation and possibly additional charge state modification by collisional or other means in the corona. A wide range of iron charge states have been measured for a variety of SEP events, ranging from =10+ to 20+. The mean charge states of C, O, Ne, Mg and Si all increased as the iron charge state increased. In events with the highest iron charge states, there were abundance enhancements in Ne with respect to oxygen in those cases, even though the mass/charge of the O and Ne were similar. In events with the lowest iron charge states, all these ions except Mg showed mean charge states generally consistent with coronal material of an equilibrium temperature of 1.3-1.6 million degrees K

  16. Laserspray ionization on a commercial atmospheric pressure-MALDI mass spectrometer ion source: selecting singly or multiply charged ions.

    Science.gov (United States)

    McEwen, Charles N; Larsen, Barbara S; Trimpin, Sarah

    2010-06-15

    Multiply charged ions, similar to those obtained with electrospray ionization, are produced at atmospheric pressure (AP) using standard MALDI conditions of laser fluence and reflective geometry. Further, the charge state can be switched to singly charged ions nearly instantaneously by changing the voltage applied to the MALDI target plate. Under normal AP-MALDI operating conditions in which a voltage is applied to the target plate, primarily singly charged ions are observed, but at or near zero volts, highly charged ions are observed for peptides and proteins. Thus, switching between singly and multiply charged ions requires only manipulation of a single voltage. As in ESI, multiple charging, produced using the AP-MALDI source, allows compounds with molecular weights beyond the mass-to-charge limit of the mass spectrometer to be observed and improves the fragmentation relative to singly charged ions. PMID:20469839

  17. Charge State Model of Solar Energetic Particles

    Science.gov (United States)

    Del Peral, L.; Pérez-Peraza, J. A.; Rodríguez Frías, M. D.

    2013-05-01

    Charge states of heavy ions in Solar Energetic Particle (SEP) events observed at the Earth's neighborhood with experiments on board satellites give us information about physical properties of plasma where acceleration occurs. SEP detection is performed near the Earth, therefore not only physical condition of the plasma source of accelerated particles have to be taken into account. We have developed a charge state model in order to explain the evolution of particle charge states under solar acceleration. Charge-interchange processes between the accelerated ions and the plasma matter in the acceleration region are considered on basis of electron loss and capture cross sections at high energies. We have applied the model to observational data from satellites measuring charge states of SEPs. In contrast with other models that use ionization and recombination cross-sections that require application of thermal equilibrium, our model assumes that the acceleration is so fast that thermal equilibrium can not be applied to the change interchange processes. Therefore we employ in our model high energy cross-sections for electron capture and loss, since the population which is being accelerated acquires a non-thermal spectrum. We have developed temperature dependent cross-sections. Acceleration begins from a thermal distribution. As soon as the particles increase their energy by the acceleration process, they acquire an energy spectrum which differs from the Maxwellian thermal one while interacting with the background thermal matter. Figure 1 presents the results of our model that fit experimental charge states of Fe ions from two impulsive SEP events detected by the SEPICA satellite in July 1999. We obtain good fitting for source temperature of 1.8 \\cdot 106 K and density of 5\\cdot108 cm-3 and acceleration efficiency of 1.8\\cdot 10-2 s-1 for the July 20th 1999 event and 3.3\\cdot 10-2 s-1 for the July 3rd 1999. Good concordance between experimental data and our model have

  18. A data-driven adaptive state of charge and power capability joint estimator of lithium-ion polymer battery used in electric vehicles

    International Nuclear Information System (INIS)

    An accurate SoC (state of charge) and SoP (state of power capability) joint estimator is the most significant techniques for electric vehicles. This paper makes two contributions to the existing literature. (1) A data-driven parameter identification method has been proposed for accurately capturing the real-time characteristic of the battery through the recursive least square algorithm, where the parameter of the battery model is updated with the real-time measurements of battery current and voltage at each sampling interval. (2) An adaptive extended Kalman filter algorithm based multi-state joint estimator has been developed in accordance with the relationship of the battery SoC and its power capability. Note that the SoC and SoP can be predicted accurately against the degradation and various operating environments of the battery through the data-driven parameter identification method. The robustness of the proposed data-driven joint estimator has been verified by different degradation states of lithium-ion polymer battery cells. The result indicates that the estimation errors of voltage and SoC are less than 1% even if given a large erroneous initial state of joint estimator, which makes the SoP estimate more accurate and reliable for the electric vehicles application. - Highlights: • A data-driven parameter identification method is developed by RLS algorithm. • An adaptive multi-state joint estimator of the battery is developed by AEKF algorithm. • A data-driven SoC and SoP joint estimator is developed with the real-time measurement. • Robustness of the joint estimator is verified by different aging states of LiPB cells

  19. Charge breeding ions for nuclear physics with the PHOENIX ECRIS

    International Nuclear Information System (INIS)

    At ISOLDE, CERN, an online PHOENIX ECR charge state breeder is being tested for the investigation of the 1+→n+ scenario for the next generation ISOL postaccelerators. As the program of tests reaches an end, the possible physics experiments with multiply charged radioactive ion beams are being investigated. Especially the use of the ECR charge breeder in combination with a high voltage platform would permit an acceleration of the radioactive ions produced at ISOLDE to total energies up to a few MeV. This opens up possibilities for nuclear astrophysics experiments such as various studies of low energy radiative capture reactions. Experiments requiring the implantation of radioactive ions in a substrate at varying depth can also be conceived. This contribution presents the various aspects of the current performances of the PHOENIX ECR charge breeder that could benefit physics applications.

  20. Ion distribution function in ion space-charge region

    International Nuclear Information System (INIS)

    Experimental results for the ion distribution functions measured into an ion space-charge region near the negatively biased grid of a multipolar confinement plasma system are presented. The ion space charge is produced in argon plasma at a pressure of about 10-4 mbar. Plasma parameters in source chamber were electron density in the range 108 to 1010 cm-3 and electron temperature in the range 0.5 to 6.0 eV. The ion distribution functions were measured using a small electrostatic analyser with two grids of about 8 mm effective diameter and 48% optical transparency. The are two regimes for ion space-charge formation: one regime is stable and another is unstable. The latter consists of large current fluctuations in external electrical circuits. The ion distribution functions for both regimes are measured and the differences between them are pointed out. In the nonstationary regime the ion distribution functions are broader than in the stationary one. This effect is more important if the distance between the grid and the electrostatic analyser is greater than the ion space-charge position. (authors)

  1. Charge-state and element-resolved ion energies in the cathodic arc plasma from composite AlCr cathodes in argon, nitrogen and oxygen atmospheres

    CERN Document Server

    Franz, Robert; Anders, André

    2014-01-01

    The energy distribution functions of ions in the cathodic arc plasma using composite AlCr cathodes were measured as a function of the background gas pressure in the range 0.5 to 3.5 Pa for different cathode compositions and gas atmospheres. The most abundant aluminium ions were Al$^{+}$ regardless of the background gas species, whereas Cr$^{2+}$ ions were dominating in Ar and N$_2$ and Cr$^{+}$ in O$_2$ atmospheres. The energy distributions of the aluminium and chromium ions typically consisted of a high energy fraction due to acceleration in the expanding plasma plume from the cathode spot and thermalised ions that were subjected to collisions in the plasma cloud. The fraction of the latter increased with increasing background gas pressure. Atomic nitrogen and oxygen ions showed similar energy distributions as the aluminium and chromium ions, whereas the argon and molecular nitrogen and oxygen ions were mainly thermalised. In addition to the positively charged metal and gas ions, negatively charged oxygen an...

  2. Analysis of the Deposit Layer from Electrolyte Side Reaction on the Anode of the Pouch Type Lithium Ion Polymer Batteries: The Effect of State of Charge and Charge Rate

    International Nuclear Information System (INIS)

    Highlights: • Raising the battery cycling potential increased the rate of side reaction. • Growth of deposit layer thickness at the electrode/electrolyte interface at high SOC. • A significant amount of lithium was consumed in forming the deposit layer. • Some of the lithium were “trapped” in the graphite after the discharge cycle. - Abstract: The formation of the solid electrolyte interface (SEI) layer on the surface of the anode electrode of a lithium ion battery prevents further electrolyte decomposition reaction. However, at certain battery operating conditions, the SEI breakdown leading to more electrolyte decomposition reactions that form several species on the anode electrode surface. This paper focuses on the effect of battery potential and charge rate on the decomposition side reaction on the anode electrode of a lithium ion polymer battery, as a result of the breakdown of the SEI layer. The results from this study indicate that raising the state of charge (SOC) increases the rate of the electrolyte decomposition side reaction that resulted in formation of a thick deposit layer at the electrolyte/electrolyte interface. This deposit layer contains lithium that can no longer participate in the reversible electrochemical reaction. In addition, at high cycling potential and charge rates the amount of lithium in the graphite after complete cell discharge increased due to the entrapment of lithium in the graphite. The amount of irreversible capacity loss for the batteries cycled at high potential and current correlates with the amount of trapped lithium in the graphite and the growth of the deposit layer thickness at the electrode/electrolyte interface

  3. Production of highly charged ion beams from electron cyclotron resonance ion sources (invited)

    International Nuclear Information System (INIS)

    Electron cyclotron resonance ion source (ECRIS) development has progressed with multiple-frequency plasma heating, higher mirror magnetic fields, and better technique to provide extra cold electrons. Such techniques greatly enhance the production of highly charged ions from ECRISs. So far at continuous wave (CW) mode operation, up to 300 eμA of O7+ and 1.15 emA of O6+, more than 100 eμA of intermediate heavy ions for charge states up to Ar13+, Ca13+, Fe13+, Co14+, and Kr18+, and tens of eμA of heavy ions with charge states to Kr26+, Xe28+, Au35+, Bi34+, and U34+ were produced from ECRISs. At an intensity of at least 1 eμA, the maximum charge state available for the heavy ions are Xe36+, Au46+, Bi47+, and U48+. An order of magnitude enhancement for fully stripped argon ions (I≥60enA) were also achieved. This article will review the ECR ion source progress and discuss key requirement for ECRISs to produce the highly charged ion beams. copyright 1998 American Institute of Physics

  4. Experimental recombination rates for highly charged ions

    International Nuclear Information System (INIS)

    Recent studies of recombination between free electrons and highly charged ions using electron coolers of heavy-ion storage rings have produced accurate rate coefficients of interest for plasma modeling and diagnostics. Some surprises were discovered which can lead to revisions of recombination models. With bare ions one finds at low energy a strong and puzzling deviation from radiative recombination theory. Dielectronic recombination with C3+, N4+) show that jj coupling gives essential contributions to the cross section also for light ions. (author)

  5. Simultaneous acceleration of multiply charged ions through a superconducting linac

    CERN Document Server

    Ostroumov, P N; Zinkann, G P; Shepard, K W; Nolen, J A

    2001-01-01

    The possibility of simultaneously accelerating particles with a range of charge-to-mass ratios (~20%) to the same energy is proposed and demonstrated for a superconducting linac. Uranium ions stripped in a foil with eight charge states have been accelerated through a portion of the ATLAS linac from 286 to 690 MeV, with 94% of the injected uranium in the accelerated beam. Emittance of the resultant beam has been measured and the energy spread was 1.3% compared to 0.4% for a single charge state. This development has immediate application to the high-intensity acceleration of heavy ions that are limited by ion-source intensities, such as the proposed rare isotope accelerator facility. (6 refs).

  6. Final state effects on charge asymmetry of pion elliptic flow in high-energy heavy-ion collisions

    International Nuclear Information System (INIS)

    Within a multi-phase transport (AMPT) model with the string melting mechanism and imported initial electric quadrupole moment, the difference between the elliptic flow of positive and negative pions is calculated. The slope parameter r of the linear dependence of Δv2=v2(π−)−v2(π+) on Ach=(N+−N−)/(N++N−) is yielded owing to the parton cascade, which converts the initial electric quadrupole distribution into the final charge-dependent elliptic flow. The slope parameter r is found to be increased by the hadronization given by the coalescence, and decreased by the resonance decays. The slope parameter r is very sensitive to both the initial electric quadrupole percentage and centrality bin and consequently a helpful constraint on the quadrupole moment of the chiral magnetic wave is obtained for Au + Au collisions at the top RHIC energy

  7. Discrete wavelet transform-based denoising technique for advanced state-of-charge estimator of a lithium-ion battery in electric vehicles

    International Nuclear Information System (INIS)

    Sophisticated data of the experimental DCV (discharging/charging voltage) of a lithium-ion battery is required for high-accuracy SOC (state-of-charge) estimation algorithms based on the state-space ECM (electrical circuit model) in BMSs (battery management systems). However, when sensing noisy DCV signals, erroneous SOC estimation (which results in low BMS performance) is inevitable. Therefore, this manuscript describes the design and implementation of a DWT (discrete wavelet transform)-based denoising technique for DCV signals. The steps for denoising a noisy DCV measurement in the proposed approach are as follows. First, using MRA (multi-resolution analysis), the noise-riding DCV signal is decomposed into different frequency sub-bands (low- and high-frequency components, An and Dn). Specifically, signal processing of the high frequency component Dn that focuses on a short-time interval is necessary to reduce noise in the DCV measurement. Second, a hard-thresholding-based denoising rule is applied to adjust the wavelet coefficients of the DWT to achieve a clear separation between the signal and the noise. Third, the desired de-noised DCV signal is reconstructed by taking the IDWT (inverse discrete wavelet transform) of the filtered detailed coefficients. Finally, this signal is sent to the ECM-based SOC estimation algorithm using an EKF (extended Kalman filter). Experimental results indicate the robustness of the proposed approach for reliable SOC estimation. - Highlights: • Sophisticated data of the experimental DCV is required for high-accuracy SOC. • DWT (discrete wavelet transform)-based denoising technique is newly investigated. • Three steps for denoising a noisy DCV measurement in this work are implemented. • Experimental results indicate the robustness of the proposed work for reliable SOC

  8. Ion accumulation and space charge neutralization in intensive electron beams for ion sources and electron cooling

    International Nuclear Information System (INIS)

    The Electron Beam Ion Sources (EBIS), Electron Beam Ion Traps (EBIT) and electron beams for electron cooling application have the beam parameters in the same ranges of magnitudes. EBIS and EBIT produce and accumulate ions in the beam due to electron impact ionization. The cooling electron beam accumulates positive ions from the residual gas in the accelerator chamber during the cooling cycle. The space charge neutralization of cooling beam is also used to reduce the electron energy spread and enhance the cooling ability. The advanced results of experimental investigations and theoretical models of the EBIS electron beams are applied to analyze the problem of beam neutralization in the electron cooling techniques. The report presents the analysis of the most important processes connected with ion production, accumulation and losses in the intensive electron beams of ion sources and electron cooling systems for proton and ion colliders. The inelastic and elastic collision processes of charged particles in the electron beams are considered. The inelastic processes such as ionization, charge exchange and recombination change the charge states of ions and neutral atoms in the beam. The elastic Coulomb collisions change the energy of particles and cause the energy redistribution among components in the electron-ion beams. The characteristic times and specific features of ionization, beam neutralization, ion heating and loss in the ion sources and electron cooling beams are determined. The dependence of negative potential in the beam cross section on neutralization factor is studied. 17 refs., 5 figs., 1 tab

  9. State of the Art ECR Ion Sources

    International Nuclear Information System (INIS)

    Electron Cyclotron Resonance (ECR) ion source which produces highly-charged ions is used in heavy ion accelerators worldwide. Applications also found in atomic physics research and industry ion implantation. ECR ion source performance continues to improve, especially in the last few years with new techniques, such as multiple-frequency plasma heating and better methods to provide extra cold electrons, combined with higher magnetic mirror fields. So far more than 1 emA of multiply-charged ions such as He2+ and O6+, and 30 eμA of Au32+, 1.1 eμA of 238U48+, and epA currents of very high charge states such as 86Kr35+ and 238U60+ have been produced

  10. Simplification of physics-based electrochemical model for lithium ion battery on electric vehicle. Part II: Pseudo-two-dimensional model simplification and state of charge estimation

    Science.gov (United States)

    Han, Xuebing; Ouyang, Minggao; Lu, Languang; Li, Jianqiu

    2015-03-01

    Now the lithium ion batteries are widely used in electric vehicles (EV). The battery modeling and state estimation are of great importance. The rigorous physics-based electrochemical model is too complicated for on-line simulation in vehicle. In this work, the simplification of the physics-based model for application on real vehicle is proposed. An improved single particle (SP) model is introduced with high precision and the same level of computations as the original single particle model. A simplified pseudo-two-dimensional (SP2D) model is developed. The distribution of the pore wall flux is analyzed and an approximate method is developed to find the solution. The developed models are compared with rigorous electrochemical model and original SP models. The results demonstrate that the models introduced in this work could simulate the battery efficiently without too much loss of accuracy. A state of charge (SOC) estimation algorithm using the Luenberger observer with the SP2D model is proposed and shows high precision. This SOC estimation method could be used in the BMS in real vehicle.

  11. Ion specific effects on charged interfaces

    OpenAIRE

    Medda, Luca

    2013-01-01

    The physico-chemical phenomena occurring at charged interfaces are specifically affected by the type and the concentration of electrolytes. This has implications both in living and in inorganic systems. The discovery of the ‘ion specific effects’ dates back to Hofmeister (1888), who observed the specific effect of salts in promoting egg white proteins precipitation. Nowadays we are aware that ion specific effects are ubiquitous in all fields of science and technology where electrolytes play a...

  12. The effective charge effect in partially stripped ion-helium collisions

    International Nuclear Information System (INIS)

    The double and single ionization cross section ratios of helium by partially stripped carbon, oxygen and fluorine ions are measured for projectile charge states ranging from +1 to +4 and impact energies from 1.5 MeV to 7.5 MeV. The effective charge effect in partially stripped ion-helium collisions is studied. It is found that the effective charge qeff increases as the impinging energy increases and qeff shows a modest dependence upon the projectile charge state in the present energy range. The projectile charge state, projectile energy, projectile and target electronic state dependences of the effective charge effect may be explained using orbital interpenetrating. (orig.)

  13. Production of Charge in Heavy Ion Collisions

    CERN Document Server

    Pratt, Scott; Ratti, Claudia

    2015-01-01

    By analyzing preliminary experimental measurements of charge-balance functions from the STAR Collaboration at the Relativistic-Heavy-Ion Collider (RHIC), it is found that pictures where balancing charges are produced in a single surge, and therefore separated by a single length scale, are inconsistent with data. In contrast, a model that assumes two surges, one associated with the formation of a thermalized quark-gluon plasma and a second associated with hadronization, provides a far superior reproduction of the data. A statistical analysis of the model comparison finds that the two-surge model best reproduces the data if the charge production from the first surge is similar to expectations for equilibrated matter taken from lattice gauge theory. The charges created in the first surge appear to separate by approximately one unit of spatial rapidity before emission, while charges from the second wave appear to have separated by approximately a half unit or less.

  14. Production of charge in heavy ion collisions

    Science.gov (United States)

    Pratt, Scott; McCormack, William Patrick; Ratti, Claudia

    2015-12-01

    By analyzing preliminary experimental measurements of charge-balance functions from the STAR Collaboration at the Relativistic Heavy Ion Collider (RHIC), it is found that scenarios in which balancing charges are produced in a single surge, and therefore separated by a single length scale, are inconsistent with data. In contrast, a model that assumes two surges, one associated with the formation of a thermalized quark-gluon plasma and a second associated with hadronization, provides a far superior reproduction of the data. A statistical analysis of the model comparison finds that the two-surge model best reproduces the data if the charge production from the first surge is similar to expectations for equilibrated matter taken from lattice gauge theory. The charges created in the first surge appear to separate by approximately one unit of spatial rapidity before emission, while charges from the second wave appear to have separated by approximately a half unit or less.

  15. State of charge estimation of lithium-ion batteries using the open-circuit voltage at various ambient temperatures

    International Nuclear Information System (INIS)

    Highlights: • An offline OCV–SOC–temperature table was established to infer battery SOC. • A temperature-based model was developed to estimate SOC at different temperatures. • The algorithm for SOC estimation was verified by dynamic current load. • The robustness of the approach was validated by different initial SOC values. - Abstract: Ambient temperature is a significant factor that influences the accuracy of battery SOC estimation, which is critical for remaining driving range prediction of electric vehicles (EVs) and optimal charge/discharge control of batteries. A widely used method to estimate SOC is based on an online inference of open-circuit voltage (OCV). However, the fact that the OCV–SOC is dependent on ambient temperature can result in errors in battery SOC estimation. To address this problem, this paper presents an SOC estimation approach based on a temperature-based model incorporated with an OCV–SOC–temperature table. The unscented Kalman filtering (UKF) was applied to tune the model parameters at each sampling step to cope with various uncertainties arising from the operation environment, cell-to-cell variation, and modeling inaccuracy. Two dynamic tests, the dynamic stress test (DST) and the federal urban driving schedule (FUDS), were used to test batteries at different temperatures. Then, DST was used to identify the model parameters while FUDS was used to validate the performance of the SOC estimation. The estimation was made covering the major working range from 25% to 85% SOC. The results indicated that our method can provide accurate SOC estimation with smaller root mean squared errors than the method that does not take into account ambient temperature. Thus, our approach is effective and accurate when battery operates at different ambient temperatures. Since the developed method takes into account the temperature factor as well as the complexity of the model, it could be effectively applied in battery management systems for

  16. Electrochemical model based charge optimization for lithium-ion batteries

    Science.gov (United States)

    Pramanik, Sourav; Anwar, Sohel

    2016-05-01

    In this paper, we propose the design of a novel optimal strategy for charging the lithium-ion battery based on electrochemical battery model that is aimed at improved performance. A performance index that aims at minimizing the charging effort along with a minimum deviation from the rated maximum thresholds for cell temperature and charging current has been defined. The method proposed in this paper aims at achieving a faster charging rate while maintaining safe limits for various battery parameters. Safe operation of the battery is achieved by including the battery bulk temperature as a control component in the performance index which is of critical importance for electric vehicles. Another important aspect of the performance objective proposed here is the efficiency of the algorithm that would allow higher charging rates without compromising the internal electrochemical kinetics of the battery which would prevent abusive conditions, thereby improving the long term durability. A more realistic model, based on battery electro-chemistry has been used for the design of the optimal algorithm as opposed to the conventional equivalent circuit models. To solve the optimization problem, Pontryagins principle has been used which is very effective for constrained optimization problems with both state and input constraints. Simulation results show that the proposed optimal charging algorithm is capable of shortening the charging time of a lithium ion cell while maintaining the temperature constraint when compared with the standard constant current charging. The designed method also maintains the internal states within limits that can avoid abusive operating conditions.

  17. Photodetachment of the negatively charged hydrogen ions

    CERN Document Server

    Frolov, Alexei M

    2015-01-01

    Photodetachment cross-sections of the negatively charged hydrogen ion(s) ${}^{\\infty}$H$^{-}$, ${}^{1}$H$^{-}$ (protium), ${}^{2}$H$^{-}$ (deuterium D$^{-}$) and ${}^{3}$H$^{-}$ (tritium T$^{-}$) are determined with the use of highly accurate, truly correlated, variational wave functions constructed for these ions. Our approach is based on some efficient and numerically stable formulas for the three-particle integrals with the Bessel functions of the first kind which have been derived recently. Application of the Rayleigh's formula for the spherical Bessel functions drastically simplifies the whole procedure and makes it numerically stable.

  18. An EBIS for charge state breeding in the SPES project

    Indian Academy of Sciences (India)

    V Variale; G Brautti; T Clauser; A Rainò; V Stagno; G Lamanna; V Valentino; A Boggia; Y Boimelshtein; P Logatchov; B Skarbo; M Tiunov

    2002-11-01

    The ‘charge state breeder’, BRIC (breeding ion charge) is in construction at the INFN section of Bari (Italy). It is based on EBIS scheme and it is designed to accept radioactive ion beam (RIB) with charge state +1 in a slow injection mode. This experiment can be considered as a first step towards the design and construction of a charge breeder for the SPES project. The new feature of BRIC, with respect to the classical EBIS, is given by the insertion, in the ion chamber, of a rf-quadrupole aiming at filtering the unwanted masses and then making a more efficient containment of the wanted ions. In this paper, the breeder design, the simulation results of the electron and ion beam propagation and the construction problems of the device will be reported.

  19. Doubly-charged Negative Ion of C60 Molecule

    OpenAIRE

    Msezane, A. Z.; Baltenkov, A S

    2016-01-01

    Within the Dirac- and Lorentz-bubble potential models an electronic structure of the doubly-charged negative ion has been studied by a variational method. It is shown that even in the first approximation of this method when a trial wave function of the two electrons is represented as a product of one-electron functions the total energy of the system is negative, a manifestation of the existence of a stable state of the doubly-charged negative ion in these models. The second electron affinity ...

  20. Doubly-charged Negative Ion of C60 Molecule

    CERN Document Server

    Msezane, A Z

    2016-01-01

    Within the Dirac- and Lorentz-bubble potential models an electronic structure of the doubly-charged negative ion has been studied by a variational method. It is shown that even in the first approximation of this method when a trial wave function of the two electrons is represented as a product of one-electron functions the total energy of the system is negative, a manifestation of the existence of a stable state of the doubly-charged negative ion in these models. The second electron affinity of C60 according to estimation is about 1 eV. The photodetachment cross sections of this ion have been calculated as well. Near threshold behavior of cross section is found to exhibit peculiar and interesting behavior. The first cross section accompanied by the transformation of the doubly-charged negative ion into a singly-charged one is exponentially small near the process threshold. The second cross section corresponds to the photodetachment of a singly-charged ion; it increases at the threshold as a power function of ...

  1. Solar Wind Charge Exchange Studies Of Highly Charged Ions On Atomic Hydrogen

    International Nuclear Information System (INIS)

    Accurate studies of low-energy charge exchange (CX) are critical to understanding underlying soft X-ray radiation processes in the interaction of highly charged ions from the solar wind with the neutral atoms and molecules in the heliosphere, cometary comas, planetary atmospheres, interstellar winds, etc.. Particularly important are the CX cross sections for bare, H-like, and He-like ions of C, N, O and Ne, which are the dominant charge states for these heavier elements in the solar wind. Absolute total cross sections for single electron capture by H-like ions of C, N, O and fully-stripped O ions from atomic hydrogen have been measured in an expanded range of relative collision energies (5 eV/u-20 keV/u) and compared to previous H-oven measurements. The present measurements are performed using a merged-beams technique with intense highly charged ion beams extracted from a 14.5 GHz ECR ion source installed on a high voltage platform at the Oak Ridge National Laboratory. For the collision energy range of 0.3 keV/u-3.3 keV/u, which corresponds to typical ion velocities in the solar wind, the new measurements are in good agreement with previous H-oven measurements. The experimental results are discussed in detail and compared with theoretical calculations where available.

  2. Review of highly charged heavy ion production with electron cyclotron resonance ion source (invited).

    Science.gov (United States)

    Nakagawa, T

    2014-02-01

    The electron cyclotron resonance ion source (ECRIS) plays an important role in the advancement of heavy ion accelerators and other ion beam applications worldwide, thanks to its remarkable ability to produce a great variety of intense highly charged heavy ion beams. Great efforts over the past decade have led to significant ECRIS performance improvements in both the beam intensity and quality. A number of high-performance ECRISs have been built and are in daily operation or are under construction to meet the continuously increasing demand. In addition, comprehension of the detailed and complex physical processes in high-charge-state ECR plasmas has been enhanced experimentally and theoretically. This review covers and discusses the key components, leading-edge developments, and enhanced ECRIS performance in the production of highly charged heavy ion beams. PMID:24593514

  3. Review of highly charged heavy ion production with electron cyclotron resonance ion source (invited)

    Science.gov (United States)

    Nakagawa, T.

    2014-02-01

    The electron cyclotron resonance ion source (ECRIS) plays an important role in the advancement of heavy ion accelerators and other ion beam applications worldwide, thanks to its remarkable ability to produce a great variety of intense highly charged heavy ion beams. Great efforts over the past decade have led to significant ECRIS performance improvements in both the beam intensity and quality. A number of high-performance ECRISs have been built and are in daily operation or are under construction to meet the continuously increasing demand. In addition, comprehension of the detailed and complex physical processes in high-charge-state ECR plasmas has been enhanced experimentally and theoretically. This review covers and discusses the key components, leading-edge developments, and enhanced ECRIS performance in the production of highly charged heavy ion beams.

  4. Review of highly charged heavy ion production with electron cyclotron resonance ion source (invited)

    International Nuclear Information System (INIS)

    The electron cyclotron resonance ion source (ECRIS) plays an important role in the advancement of heavy ion accelerators and other ion beam applications worldwide, thanks to its remarkable ability to produce a great variety of intense highly charged heavy ion beams. Great efforts over the past decade have led to significant ECRIS performance improvements in both the beam intensity and quality. A number of high-performance ECRISs have been built and are in daily operation or are under construction to meet the continuously increasing demand. In addition, comprehension of the detailed and complex physical processes in high-charge-state ECR plasmas has been enhanced experimentally and theoretically. This review covers and discusses the key components, leading-edge developments, and enhanced ECRIS performance in the production of highly charged heavy ion beams

  5. Argon-ion charge distributions following near-threshold ionization

    International Nuclear Information System (INIS)

    When an atom is photoionized in an inner shell, there are two mechanisms by which the remaining electron cortege relaxes to fill the vacancy: x-ray emission and radiationless Auger and Coster-Kronig transitions. In the former, the inner-shell hole moves to a less tightly bound orbital without increasing the number of atomic vacancies. In Auger processes, however, the energy liberated by transfer of a less-tightly-bound electron to the inner-shell vacancy is transferred to another electron which is ejected into the continuum. In this case, the charge on the residual ion increases by one. Through a series of radiative and non-radiative processes, the initial vacancy bubbles up until all vacancies arrive at the outermost shell. Due to the many possible routes by which this may occur, there can be a broad distribution of residual ion charge states characteristic of the decay of a single inner-shell vacancy. Because so many processes can contribute to each charge state, it is difficult to determine the effect of each by examining the total ion charge distribution; the total-ion charge distribution represents an average over many effects. To overcome this limitation, the author has recently measured argon-ion production as a function of both photon energy and Auger decay channel following photoionization of K-shell electrons with highly monochromatic synchrotron radiation. When measured differential in decay channel, the ion charge distributions are greatly simplified. Analysis, in progress, of these simplified distributions will permit extraction of information about relative decay rates and shakeoff effects that is obscured in the single spectra

  6. Influence of memory effect on the state-of-charge estimation of large-format Li-ion batteries based on LiFePO4 cathode

    Science.gov (United States)

    Shi, Wei; Wang, Jiulin; Zheng, Jianming; Jiang, Jiuchun; Viswanathan, Vilayanur; Zhang, Ji-Guang

    2016-04-01

    In this work, we systematically investigated the influence of the memory effect of LiFePO4 cathodes in large-format full batteries. The electrochemical performance of the electrodes used in these batteries was also investigated separately in half-cells to reveal their intrinsic properties. We noticed that the memory effect of LiFePO4/graphite cells depends not only on the maximum state of charge reached during the memory writing process, but is also affected by the depth of discharge reached during the memory writing process. In addition, the voltage deviation in a LiFePO4/graphite full battery is more complex than in a LiFePO4/Li half-cell, especially for a large-format battery, which exhibits a significant current variation in the region near its terminals. Therefore, the memory effect should be taken into account in advanced battery management systems to further extend the long-term cycling stabilities of Li-ion batteries using LiFePO4 cathodes.

  7. State of charge estimation of Li-ion batteries in an electric vehicle based on a radial-basis-function neural network

    International Nuclear Information System (INIS)

    The on-line estimation of the state of charge (SOC) of the batteries is important for the reliable running of the pure electric vehicle in practice. Because a nonlinear feature exists in the batteries and the radial-basis-function neural network (RBF NN) has good characteristics to solve the nonlinear problem, a practical method for the SOC estimation of batteries based on the RBF NN with a small number of input variables and a simplified structure is proposed. Firstly, in this paper, the model of on-line SOC estimation with the RBF NN is set. Secondly, four important factors for estimating the SOC are confirmed based on the contribution analysis method, which simplifies the input variables of the RBF NN and enhances the real-time performance of estimation. Finally, the pure electric buses with LiFePO4 Li-ion batteries running during the period of the 2010 Shanghai World Expo are considered as the experimental object. The performance of the SOC estimation is validated and evaluated by the battery data from the electric vehicle

  8. Challenges and requirements of charge state monitoring of lithium ion batteries; Anforderungen und Herausforderungen bei der Zustandsbestimmung von Lithium-Ionen Batterien

    Energy Technology Data Exchange (ETDEWEB)

    Sauer, Dirk Uwe; Gerschler, Jochen B.; Sinhuber, Philipp [RWTH Aachen (Germany). ISEA

    2010-07-01

    Lithium-Ion batteries are a keystone for electro mobility concepts. Energy and power density as well as cycle lifetimes are superior to all other currently commercially available rechargeable battery technologies. However, generalised statements are difficult because of a large variety of different electrode materials and electrolyte which are used in commercial products. A special feature of all materials is the fact, that no standard side reaction is available which can take up surplus charging current without destroying the battery cell. If a cell is overcharged, the surplus current goes right away into an ageing process and may result in a disintegration of the electrode materials and finally in a thermal runaway of the cells. The huge variety in material combinations as well as the missing side reaction have a strong impact on the determination of the state of function. Algorithms and concepts need to be adapted in every single case to the specific properties of the used materials. Further more, the performance of the battery system is determined by the weakest cell in the battery system. Therefore supervision and an analysis of each cell are necessary. (orig.)

  9. Fuzzy Sliding Mode Observer with Grey Prediction for the Estimation of the State-of-Charge of a Lithium-Ion Battery

    Directory of Open Access Journals (Sweden)

    Daehyun Kim

    2015-11-01

    Full Text Available We propose a state-of-charge (SOC estimation method for Li-ion batteries that combines a fuzzy sliding mode observer (FSMO with grey prediction. Unlike the existing methods based on a conventional first-order sliding mode observer (SMO and an adaptive gain SMO, the proposed method eliminates chattering in SOC estimation. In this method, which uses a fuzzy inference system, the gains of the SMO are adjusted according to the predicted future error and present estimation error of the terminal voltage. To forecast the future error value, a one-step-ahead terminal voltage prediction is obtained using a grey predictor. The proposed estimation method is validated through two types of discharge tests (a pulse discharge test and a random discharge test. The SOC estimation results are compared to the results of the conventional first-order SMO-based and the adaptive gain SMO-based methods. The experimental results show that the proposed method not only reduces chattering, but also improves estimation accuracy.

  10. A space charge compensation model for positive DC ion beams

    International Nuclear Information System (INIS)

    In this paper, we revisit and extend a formula to predict the compensation of space charge in positive DC ion beams of non-relativistic energy, as they are for example found in the injector beam lines of heavy ion accelerator facilities.The original formula was presented in 1975 by Igor Gabovich et al. and takes into account the de-compensation through Coulomb collisions of the primary beam ions and the compensating electrons. We extend its usability to arbitrary (positive) charge states of the ions and non-quasineutral beams.The resulting formula compares well with measurements using a retarding field analyzer and a multi-species generalization of it was incorporated into beam transport simulations using the particle-in-cell code WARP

  11. Cluster ions and multiply charged ions formed in frozen CO2 molecules under heavy ion impact

    International Nuclear Information System (INIS)

    A variety of cluster ions, positive or negative, as well as multiply charged atomic ions have been observed from the frozen CO2 targets under (MeV/amu) energetic, highly charged projectile ion impact. Their spectra are found to be quite different from those produced in the cooled expanding CO2 gas targets

  12. Electron impact single ionisation of multiply charged krypton ions

    International Nuclear Information System (INIS)

    Absolute cross sections σsub(q,q+1) for electron impact single ionisation of Krsup(q+) ions (q = 1, 2, 3) have been measured for electron energies up to 700 eV by employing a dynamic crossed-beams technique. The experimental data significantly exceed the Lotz prediction for direct ionisation of Kr2+ and Kr3+ ions, indicating the importance of indirect processes for multiply charged Krsup(q+) ions. The observed ionisation thresholds of cross sections from the present measurements as well as of data from other workers indicate the presence of metastable ions in the parent ion beams. The influence of metastable states on the cross sections is discussed on the basis of Lotz calculations for direct ionisation from different excited states, and differences observed in the experiments are rationalised. (author)

  13. Measurement of charge exchange cross sections for highly charged xenon and thorium ions with molecular hydrogen in a Penning Ion Trap

    Energy Technology Data Exchange (ETDEWEB)

    Weinberg, G.M.

    1995-12-01

    Highly charged xenon (35+ to 46+) and thorium (72+ to 79+) ions were produced in an Electron Beam Ion Trap (EBIT). The ions were extracted from EBIT in a short pulse. Ions of one charge state were selected using an electromagnet. The ions were recaptured at low energy in a cryogenic Penning trap (RETRAP). As the ions captured electrons from molecular hydrogen, populations of the various charge states were obtained by measuring the image currents induced by the ions on the electrodes of the trap. Data on the number of ions in each charge state vs. time were compared to theoretical rate equations in order to determine the average charge exchange rates. These rates were compared to charge exchange rates of an ion with a known charge exchange cross section (Ar{sup 11+}) measured in a similar manner in order to determine the average charge exchange cross sections for the highly charged ions. The energy of interaction between the highly charged ions and hydrogen was estimated to be 4 eV in the center of mass frame. The mean charge exchange cross sections were 9 {times} 10{sup {minus}14} cm{sup 2} for Xe{sup 43+} to Xe{sup 46+} and 2 {times} 10{sup {minus}13} cm{sup 2} for Th{sup 73+} to Th{sup 79+}. Double capture was approximately 20--25% of the total for both xenon and thorium. A fit indicated that the cross sections were approximately proportional to q. This is consistent with a linear dependence of cross section on q within the measurement uncertainties.

  14. Pragmatic development of a laser ion source for intense highly-charged ion beam

    International Nuclear Information System (INIS)

    Recently, applications of high-charge-state (including fully stripped) heavy-ion beams have been attracting interest in both physics and industry. To enhance their usefulness, more intense beams are required. Cancer therapy using carbon ions is a particularly promising heavy-ion beam application. Due to advances in laser technology, the laser ion source (LIS) has become one of the most popular sources for generating highly charged and intense heavy-ion beams. The project to develop a high-intensity LIS was started on June 2009. In our project, whose ultimate goal is to apply a heavy-ion accelerator for cancer therapy, we have almost completed designing the LIS, and manufacturing will commence soon. We intend to measure the source performance by performing plasma and beam tests up until the end of March 2011. We will report the outline and a progress of the project. (author)

  15. Interaction of slow highly charged ions with surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Haake, Christian; Peters, Thorsten; Wucher, Andreas; Schleberger, Marika [Universitaet Duisburg-Essen, Duisburg (Germany)

    2008-07-01

    A new ion beam installation has been built to investigate the mechanisms of energy dissipation in a substrate after the impact of highly charged ions. First experiments at the TU Wien made successful use of metal-insulator-metal (MIM) junctions to measure electronic excitations in the irradiated metal. These MIM-junctions offer the unique possibility to detect excitations below the work function which limits the external emission of electrons. In order to separate effects induced by either the kinetic or the potential energy of the projectile, both contributions need to be controlled independently. In the Vienna experiment the ions had medium charge states of q=1 up to to q=8 and kinetic energies of 400 eV to 12 keV. The new set-up offers higher charge states and is designed for kinetic energies of less than 100 eV/q. This will enable us to produce extremely slow highly charged ions. In addition, external electron emission as well as secondary and neutral mass spectrometry (SIMS/SNMS) will be used to follow the external pathways of energy dissipation.

  16. Plasma as a high-charge-state projectile stripping medium

    International Nuclear Information System (INIS)

    The classical trajectory Monte Carlo model has been used to computationally study the charge-state distributions that result from interactions between a high-energy, multielectron projectile and neutral and fully ionized targets. These studies are designed to determine the properties of a plasma for producing highly stripped ions as a possible alternative to gas and foil strippers that are commonly used to enhance the charge states of energetic ion beams. The results of these studies clearly show that a low-atomic-number, highly ionized plasma can yield higher charge states than a neutral target of the same density. The effect is principally attributable to the reduction in the number of available electron-capture channels. In this article, we compare the charge-state distributions that result during passage of a 20-MeV Pb projectile through neutral gas and fully ionized (singly charged) plasma strippers and estimate the effects of multiple scattering on the quality of the beam

  17. Laser production of highly charged ions

    Czech Academy of Sciences Publication Activity Database

    Láska, Leoš; Badziak, J.; Boody, F. P.; Gammino, S.; Jungwirth, Karel; Krása, Josef; Pfeifer, Miroslav; Rohlena, Karel; Ullschmied, Jiří; Parys, P.; Wolowski, J.; Woryna, E.; Torrisi, L.

    2005-01-01

    Roč. 34, 4B (2005), s. 1615-1619. ISSN 0103-9733 R&D Projects: GA AV ČR(CZ) IAA1010105; GA MŠk(CZ) LN00A100 Grant ostatní: EU(Projects PALS/005 and PALS/006)(XE) HPRI-CT-1999-00053; INFN(IT) ECLISSE and PLAIA Institutional research plan: CEZ:AV0Z10100523 Keywords : laser ion generation * highly charged ions * laser beam self-focusing Subject RIV: BH - Optics, Masers, Lasers Impact factor: 0.445, year: 2005

  18. Charge Exchange Collisions between Ultracold Fermionic Lithium Atoms and Calcium Ions

    CERN Document Server

    Haze, Shinsuke; Saito, Ryoichi; Mukaiyama, Takashi

    2014-01-01

    An observation of charge exchange collisions between ultracold fermionic 6Li atoms and 40Ca+ ions is reported. The reaction product of the charge exchange collision is dentified via mass spectrometry where the motion of the ions is excited parametrically. We measure the cross section of the charge exchange collisions between the 6Li atoms in the ground state and the 40Ca+ ions in the ground and metastable excited states. Investigation of the inelastic collision characteristics in the atom-ion mixture is an important step toward ultracold chemistry based on ultracold atoms and ions.

  19. Photoinduced Charge Separation in Porphyrin Ion Pairs.

    Science.gov (United States)

    Natali, Mirco; Scandola, Franco

    2016-03-10

    Ion pairs between porphyrin-type compounds have been successfully employed for spectral sensitization of semiconductor surfaces and for the preparation of collective binary ionic materials for photonic and (photo)catalytic applications. The understanding of the photophysical processes occurring within ion-paired porphyrin dimers is thus of remarkable importance for the optimization and improvement of such systems. Herein the ion-pair species formed between ZnTMePyP(4+) (Zn1) or H2TMePyP(4+) (H21) and ZnTPPS(4-) (Zn2) or H2TPPS(4-) (H22) in a variety of solvent mixtures are characterized and their photophysics thoroughly investigated by time-resolved techniques. In all the systems studied, very fast and efficient photoinduced charge separation is observed, with the cationic porphyrin being reduced and the anionic one oxidized. Interestingly, despite the very short charge separation distance, the lifetime for charge recombination, depending on the energy gap, can extend into the nanosecond time domain, showing great potential for the utilization of this molecular design within energy conversion schemes. PMID:26905260

  20. Development of 14.5 GHz Electron Cyclotron Resonance Ion Source for Muti-charged Ion Beams

    International Nuclear Information System (INIS)

    Ion sources to make multi-charged ion beam based on the electron cyclotron resonance (ECR) principle have played major role in the advancement of the knowledge of atomic and nuclear physics and in many areas of applied science and technology. Since the final energy of an ion beam is directly proportional to the charge of the ion during acceleration, a premium is placed on ion sources which are capable of generating very high charge state ion beams for use at accelerator-based research facilities. Recently in KAERI a 14.5 GHz ECRIS (Electron Cyclotron Resonance Ion Source) has been designed and is being fabricated to produce multi-charged ion beams for medical applications in a cyclotron. The design results, fabrication status, and future plan will be presented in this topic

  1. Charge stripping effects from highly charged iodine ions formed from Coulomb explosion of CH3I clusters

    International Nuclear Information System (INIS)

    Iodine ions of high charge states are observed upon irradiation of methyl iodide clusters with an intense femtosecond laser pulse. All signals from multicharged ions exhibit a peak splitting in the time-of-flight mass spectra, indicating their origin from a Coulomb explosion process. These main peaks are accompanied by smaller peaks attributed to field ionization of highly charged species in the ion optics of the TOF mass spectrometer. It is shown that highly charged atomic ions formed from Coulomb explosion, upon interaction with electric field close to the mesh, can lose another electron leading to the formation of even higher charged species. The observation of this charge stripping process is evidence for the formation of highly excited ions in the course of the Coulomb explosion process, providing new insights into the mechanisms of femtosecond ionization involving multi-electron loss. (Copyright (c) 1998 Elsevier Science B.V., Amsterdam. All rights reserved.)

  2. Correlated charge-changing ion-atom collisions

    International Nuclear Information System (INIS)

    This report summarizes the progress and accomplishments in accelerator atomic physics research supported by DOE grant DE-FG02-87ER13778 from March 16, 1991 through March 15, 1992. This work involves the experimental investigation of fundamental atomic processes in collisions of charged projectiles with neutral targets or electrons, with particular emphasis on two-electron interactions and electron correlation effects. Processes involving combinations of excitation, ionization, and charge transfer are investigated utilizing coincidence techniques in which projectiles charge-changing events are associated with x-ray emission, target recoil ions, or electron emission. New results have been obtained for studies involving (1) resonant recombination of atomic ions, (2) double ionization of helium, and (3) continuum electron emission. Experiments were conducted using accelerators at the Lawrence Berkeley Laboratory, Argonne National Laboratory, Michigan State University, Western Michigan University, and the Institute of Nuclear Research, Debrecen, Hungary. Brief summaries of work completed and work in progress are given in this report

  3. Formation and fragmentation of quadruply charged molecular ions by intense femtosecond laser pulses.

    Science.gov (United States)

    Yatsuhashi, Tomoyuki; Nakashima, Nobuaki

    2010-07-22

    We investigated the formation and fragmentation of multiply charged molecular ions of several aromatic molecules by intense nonresonant femtosecond laser pulses of 1.4 mum with a 130 fs pulse duration (up to 2 x 10(14) W cm(-2)). Quadruply charged states were produced for 2,3-benzofluorene and triphenylene molecular ion in large abundance, whereas naphthalene and 1,1'-binaphthyl resulted only in up to triply charged molecular ions. The laser wavelength was nonresonant with regard to the electronic transitions of the neutral molecules, and the degree of fragmentation was strongly correlated with the absorption of the singly charged cation radical. Little fragmentation was observed for naphthalene (off-resonant with cation), whereas heavy fragmentation was observed in the case of 1,1'-binaphthyl (resonant with cation). The degree of H(2) (2H) and 2H(2) (4H) elimination from molecular ions increased as the charge states increased in all the molecules examined. A striking difference was found between triply and quadruply charged 2,3-benzofluorene: significant suppression of molecular ions with loss of odd number of hydrogen was observed in the quadruply charged ions. The Coulomb explosion of protons in the quadruply charged state and succeeding fragmentation resulted in the formation of triply charged molecular ions with an odd number of hydrogens. The hydrogen elimination mechanism in the highly charged state is discussed. PMID:20578764

  4. Strong-field relativistic processes in highly charged ions

    International Nuclear Information System (INIS)

    In this thesis we investigate strong-field relativistic processes in highly charged ions. In the first part, we study resonance fluorescence of laser-driven highly charged ions in the relativistic regime by solving the time-dependent master equation in a multi-level model. Our ab initio approach based on the Dirac equation allows for investigating highly relativistic ions, and, consequently, provides a sensitive means to test correlated relativistic dynamics, bound-state quantum electrodynamic phenomena and nuclear effects by applying coherent light with x-ray frequencies. Atomic dipole or multipole moments may be determined to unprecedented accuracy by measuring the interference-narrowed fluorescence spectrum. Furthermore, we investigate the level structure of heavy hydrogenlike ions in laser beams. Interaction with the light field leads to dynamic shifts of the electronic energy levels, which is relevant for spectroscopic experiments. We apply a fully relativistic description of the electronic states by means of the Dirac equation. Our formalism goes beyond the dipole approximation and takes into account non-dipole effects of retardation and interaction with the magnetic field components of the laser beam. We predicted cross sections for the inter-shell trielectronic recombination (TR) and quadruelectronic recombination processes which have been experimentally confirmed in electron beam ion trap measurements, mainly for C-like ions, of Ar, Fe and Kr. For Kr30+, inter-shell TR contributions of nearly 6% to the total resonant photorecombination rate were found. (orig.)

  5. Strong-field relativistic processes in highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Postavaru, Octavian

    2010-12-08

    In this thesis we investigate strong-field relativistic processes in highly charged ions. In the first part, we study resonance fluorescence of laser-driven highly charged ions in the relativistic regime by solving the time-dependent master equation in a multi-level model. Our ab initio approach based on the Dirac equation allows for investigating highly relativistic ions, and, consequently, provides a sensitive means to test correlated relativistic dynamics, bound-state quantum electrodynamic phenomena and nuclear effects by applying coherent light with x-ray frequencies. Atomic dipole or multipole moments may be determined to unprecedented accuracy by measuring the interference-narrowed fluorescence spectrum. Furthermore, we investigate the level structure of heavy hydrogenlike ions in laser beams. Interaction with the light field leads to dynamic shifts of the electronic energy levels, which is relevant for spectroscopic experiments. We apply a fully relativistic description of the electronic states by means of the Dirac equation. Our formalism goes beyond the dipole approximation and takes into account non-dipole effects of retardation and interaction with the magnetic field components of the laser beam. We predicted cross sections for the inter-shell trielectronic recombination (TR) and quadruelectronic recombination processes which have been experimentally confirmed in electron beam ion trap measurements, mainly for C-like ions, of Ar, Fe and Kr. For Kr{sup 30}+, inter-shell TR contributions of nearly 6% to the total resonant photorecombination rate were found. (orig.)

  6. Investigation and optimization of parameters affecting the multiply charged ion yield in AP-MALDI MS.

    Science.gov (United States)

    Ryumin, Pavel; Brown, Jeffery; Morris, Michael; Cramer, Rainer

    2016-07-15

    Liquid matrix-assisted laser desorption/ionization (MALDI) allows the generation of predominantly multiply charged ions in atmospheric pressure (AP) MALDI ion sources for mass spectrometry (MS) analysis. The charge state distribution of the generated ions and the efficiency of the ion source in generating such ions crucially depend on the desolvation regime of the MALDI plume after desorption in the AP-to-vacuum inlet. Both high temperature and a flow regime with increased residence time of the desorbed plume in the desolvation region promote the generation of multiply charged ions. Without such measures the application of an electric ion extraction field significantly increases the ion signal intensity of singly charged species while the detection of multiply charged species is less dependent on the extraction field. In general, optimization of high temperature application facilitates the predominant formation and detection of multiply charged compared to singly charged ion species. In this study an experimental set-up and optimization strategy is described for liquid AP-MALDI MS which improves the ionization efficiency of selected ion species up to 14 times. In combination with ion mobility separation, the method allows the detection of multiply charged peptide and protein ions for analyte solution concentrations as low as 2fmol/μL (0.5μL, i.e. 1fmol, deposited on the target) with very low sample consumption in the low nL-range. PMID:26827934

  7. The uses of electron beam ion traps in the study of highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Knapp, D.

    1994-11-02

    The Electron Beam Ion Trap (EBIT) is a relatively new tool for the study of highly charged ions. Its development has led to a variety of new experimental opportunities; measurements have been performed with EBITs using techniques impossible with conventional ion sources or storage rings. In this paper, I will highlight the various experimental techniques we have developed and the results we have obtained using the EBIT and higher-energy Super-EBIT built at the Lawrence Livermore National Laboratory. The EBIT employs a high-current-density electron beam to trap, ionize, and excite a population of ions. The ions can be studied in situ or extracted from the trap for external experiments. The trapped ions form an ionization-state equilibrium determined by the relative ionization and recombination rates. Ions of several different elements may simultaneously be present in the trap. The ions are nearly at rest, and, for most systems, all in their ground-state configurations. The electron-ion interaction energy has a narrow distribution and can be varied over a wide range. We have used the EBIT devices for the measurement of electron-ion interactions, ion structure, ion-surface interactions, and the behavior of low-density plasmas.

  8. Charging state of atmospheric nanoparticles during the nucleation burst events

    Science.gov (United States)

    Vana, M.; Tamm, E.; Hõrrak, U.; Mirme, A.; Tammet, H.; Laakso, L.; Aalto, P. P.; Kulmala, M.

    2006-12-01

    In this work, the charging state of atmospheric nanoparticles was estimated through simultaneous measurements of aerosol size distribution and air ions mobility distribution with the aim to elucidate the formation mechanisms of atmospheric aerosols. The measurements were performed as a part of the QUEST 2 campaign at a boreal forest station in Finland. The overlapping part of the measurement ranges of the particle size spectrometers and air ion mobility spectrometers in the mass diameter interval of 2.6-40 nm was used to assess the percentage of charged particles (charging probability). This parameter was obtained as the slope of the linear regression line on the scatterplot of the measured concentrations of total (neutral + charged) and charged particles for the same diameter interval. Charging probabilities as a function of particle diameter were calculated for different days and were compared with the steady state charging probabilities of the particles in the bipolar ion atmosphere. For the smallest particles detectable by the particle size spectrometers (2.6-5 nm), the high percentages of negatively charged particles were found during the nanometer particle concentration bursts. These values considerably exceeded the values for the steady charging state and it was concluded that negative cluster ions preferably act as condensation nuclei. This effect was found to be the highest in the case of comparatively weak nucleation bursts of nanoparticles, when the rate of the homogeneous nucleation and the concentration of freshly nucleated particles were low. The nucleation burst days were classified according to the concentration of the generated smallest detectable new particles (weak and strong bursts). Approximately the same classification was obtained based on the charge asymmetry on particles with respect to the charge sign (polarity). The probabilities of negative and positive charge on the particles with the diameter of 5-20 nm were found to be nearly equal

  9. Application of carbon stripping foil to HIRFL-CSR and measurement of charge state distribution

    International Nuclear Information System (INIS)

    Charged ions may be injected into the CSRm by means of the charge stripping injection or the multiple multi-turn injection. The charge state distribution of the ions passing through the carbon foil has great influence on the performance of the accelerator and thus plays a key role in the charge stripping injection. It's found that the charge state distribution is dependent on the thicknesses of the carbon foil and the energy of the ions. In present work, the carbon stripper was applied to HIRFL-CSR and the best optional charge state distribution was measured. (authors)

  10. Progress in quantum electrodynamics theory of highly charged ions

    OpenAIRE

    Volotka, A. V.; Glazov, D. A.; Plunien, G.; Shabaev, V. M.

    2013-01-01

    Recent progress in quantum electrodynamics (QED) calculations of highly charged ions is reviewed. The theoretical predictions for the binding energies, the hyperfine splittings, and the g factors are presented and compared with available experimental data. Special attention is paid to tests of bound-state QED at strong field regime. Future prospects for tests of QED at the strongest electric and magnetic fields as well as for determination of the fine structure constant and the nuclear magnet...

  11. Calculating method for confinement time and charge distribution of ions in electron cyclotron resonance sources

    Energy Technology Data Exchange (ETDEWEB)

    Dougar-Jabon, V.D. [Escuela de Fisica, Universidad Industrial de Santander, A.A. 678, Bucaramanga (Colombia); Umnov, A.M. [Russian Friendship University, 117198 Moscow (Russia); Kutner, V.B. [Joint Institute for Nuclear Research, Dubna (Russia)

    1996-03-01

    It is common knowledge that the electrostatic pit in a core plasma of electron cyclotron resonance sources exerts strict control over generation of ions in high charge states. This work is aimed at finding a dependence of the lifetime of ions on their charge states in the core region and to elaborate a numerical model of ion charge dispersion not only for the core plasmas but for extracted beams as well. The calculated data are in good agreement with the experimental results on charge distributions and magnitudes for currents of beams extracted from the 14 GHz DECRIS source. {copyright} {ital 1996 American Institute of Physics.}

  12. Creation of surface nanostructures in Al2O3 by slow highly charged ions

    International Nuclear Information System (INIS)

    Al2O3 single crystals were irradiated with slow highly charged Xe ions of various charge states from an EBIT (Electron Beam Ion Trap) source at the Dresden two source facility. The irradiations were performed at room temperature and under normal incidence. Scanning force microscopy (SFM) was utilized to investigate the topography of the irradiated surfaces. The measurements showed that above a potential energy threshold, each ion creates a nanohillock protruding from the surface. These structures are compared to those created by swift heavy ions (SHI). The results are discussed in terms of potential energy deposition of highly charged ions (HCI) and electronic energy loss of SHI

  13. Creation of surface nanostructures in Al2O3 by slow highly charged ions

    Science.gov (United States)

    El-Said, A. S.; Wilhelm, R. A.; Heller, R.; Akhmadaliev, Sh.; Facsko, S.

    2013-12-01

    Al2O3 single crystals were irradiated with slow highly charged Xe ions of various charge states from an EBIT (Electron Beam Ion Trap) source at the Dresden two source facility. The irradiations were performed at room temperature and under normal incidence. Scanning force microscopy (SFM) was utilized to investigate the topography of the irradiated surfaces. The measurements showed that above a potential energy threshold, each ion creates a nanohillock protruding from the surface. These structures are compared to those created by swift heavy ions (SHI). The results are discussed in terms of potential energy deposition of highly charged ions (HCI) and electronic energy loss of SHI.

  14. Highly-charged ions as a basis of optical atomic clockwork of exceptional accuracy

    OpenAIRE

    Derevianko, Andrei; Dzuba, V. A.; Flambaum, V. V.

    2012-01-01

    We propose a novel class of atomic clocks based on highly charged ions. We consider highly-forbidden laser-accessible transitions within the $4f^{12}$ ground-state configurations of highly charged ions. Our evaluation of systematic effects demonstrates that these transitions may be used for building exceptionally accurate atomic clocks which may compete in accuracy with recently proposed nuclear clock.

  15. Progress in quantum electrodynamics theory of highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Volotka, Andrey V. [Institut fuer Theoretische Physik, Technische Universitaet Dresden, Mommsenstrasse 13, 01062, Dresden (Germany); Department of Physics, St. Petersburg State University, Oulianovskaya 1, Petrodvorets, 198504, St. Petersburg (Russian Federation); Glazov, Dmitry A.; Shabaev, Vladimir M. [Department of Physics, St. Petersburg State University, Oulianovskaya 1, Petrodvorets, 198504, St. Petersburg (Russian Federation); Plunien, Guenter [Institut fuer Theoretische Physik, Technische Universitaet Dresden, Mommsenstrasse 13, 01062, Dresden (Germany)

    2013-09-15

    Recent progress in quantum electrodynamics (QED) calculations of highly charged ions is reviewed. The theoretical predictions for the binding energies, the hyperfine splittings, and the g factors are presented and compared with available experimental data. Special attention is paid to tests of bound-state QED at strong field regime. Future prospects for tests of QED at the strongest electric and magnetic fields as well as for determination of the fine structure constant and the nuclear magnetic moments with heavy ions are discussed. (copyright 2013 by WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  16. Activation energies for gas-phase dissociations of multiply charged ions from electrospay ionization mass spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    Busman, M.; Rockwood, A.L.; Smith, R.D. [Pacific Northwest Lab., Richland, WA (United States)

    1992-03-19

    The reactions of multiply protonated melittin molecular ions of various charge states produced from an electrospray ionization source have been studied. The flow of ions entrained in gas through a heated metal capillary inlet serves as a reaction vessel for gas-phase measurements of molecular ion reaction rates using mass spectrometry. Activation energies for the unimolecular dissociation reactions are calculated from the temperature dependence of the reaction kinetics. The differences in activation energies for the reactions of the different charge states are attributed to the destabilizing effect of Coulombic repulsion for high charged ions. 18 refs., 3 figs., 1 tab.

  17. Charge transfer reaction of multi-charged oxygen ions with O2

    Science.gov (United States)

    Holzscheiter, H. M.; Church, D. A.

    1981-10-01

    The reaction rates for charge transfer from O2 to doubly and triply charged oxygen atoms are measured in a demonstration of the measurement capabilities of a system at ultrahigh vacuum with low-energy magnetically confined ions. Ions were produced by electron impact ionization of gas within a Penning-type ion trap, with selective removal of unwanted ionization states by radio-frequency resonant excitation. Ion number mass-to-charge ratio spectra obtained at partial pressures of O2 from 9.9 x 10 to the -9th to 1.5 x 10 to the -7th torr yield rate constants of 1.0 x 10 to the -9th cu cm/sec and 2.5 x 10 to the -9th cu cm/sec for the O(2+) and O(3+) reactions, respectively. Measurements made at a 30% increase of the effective axial well depth of the trap demonstrate that the rate constant is essentially energy independent in the energy range studies, implying that the O(2+) cross section for charge transfer has an inverse velocity dependence of the Langevin type, despite a reaction rate lower than the Langevin valve.

  18. Electron-impact single-ionization of singly and multiply charged tungsten ions

    International Nuclear Information System (INIS)

    Employing the 'crossed-beams' technique, electron-impact ionization cross sections for the single-ionization of Wq+ ions in charge states q = 1...10 have been measured. The cross sections for the ionization of ions in charge states q ≥ 5 show significant contributions below the ground-state threshold caused by the ionization of ions in excited, long-lived metastable states in the parent ion beam. In the case of W6+, the measured cross section is completely dominated by metastable contributions. For ions in charge states q = 3...7, excitation-autoionization from the ground state as well as from excited, metastable states contributes strongly to the cross sections. This results in a strong underestimation of the measured cross sections by the semiempirical Lotz formula in the energy range between the ionization threshold and the cross section maximum. (Author)

  19. Charge-transfer cross sections of ground state He+ ions in collisions with He atoms and simple molecules in the energy range below 4.0 keV

    International Nuclear Information System (INIS)

    Charge-transfer cross sections of the ground state He+ ions in collisions with He atoms and simple molecules (H2, D2, N2, CO and CO2) have been measured in the energy range of 0.20 to 4.0 keV with the initial growth rate method. Since previously published experimental data are scattered in the low energy region, the present observations would provide reasonably reliable cross section data below 4 keV. The charge transfer accompanied by dissociation of product molecular ion can be dominant at low energies for molecular targets. In He+ + D2 collisions, any isotope effect was not observed over the present energy range, compared to H2 molecule. (author)

  20. The Solar Connection of Enhanced Heavy Ion Charge States in the Interplanetary Medium: Implications for the Flux-rope Structure of CMEs

    CERN Document Server

    Gopalswamy, N; Akiyama, S; Xie, H; Yashiro, S; Reinard, A A

    2012-01-01

    We investigated a set of 54 interplanetary coronal mass ejection (ICME) events whose solar sources are very close to the disk center (within 15 degrees from the central meridian). The ICMEs consisted of 23 magnetic cloud (MC) events and 31 non-MC events. Our analyses suggest that the MC and non-MC ICMEs have more or less the same eruption characteristics at the Sun in terms of soft X-ray flares and CMEs. Both types have significant enhancements in charge states, although the non-MC structures have slightly lower levels of enhancement. The overall duration of charge state enhancement is also considerably smaller than that than that in MCs as derived from solar wind plasma and magnetic signatures. We find very good correlation between the Fe and O charge state measurements and the flare properties such as soft X-ray flare intensity and flare temperature for both MCs and non-MCs. These observations suggest that both MC and non-MC ICMEs are likely to have a flux-rope structure and the unfavorable observational ge...

  1. Influence of the density of states on the odd-even staggering in the charge distribution of the emitted fragments in nuclear heavy-ion collisions

    Science.gov (United States)

    Calleya, N. L.; Souza, S. R.; Carlson, B. V.; Donangelo, R.; Lynch, W. G.; Tsang, M. B.; Winkelbauer, J. R.

    2014-11-01

    The fragmentation of thermalized sources is studied using a version of the Statistical Multifragmentation Model which employs state densities that take the pairing gap in the nuclear levels into account. Attention is focused on the properties of the charge distributions observed in the breakup of the source. Since the microcanonical version of the model used in this study provides the primary fragment excitation energy distribution, one may correlate the reduction of the odd-even staggering in the charge distribution with the increasing occupation of high-energy states. Thus, in the framework of this model, such staggering tends to disappear as a function of the total excitation energy of the source, although the energy per particle may be small for large systems. We also find that, although the deexcitation of the primary fragments should, in principle, blur these odd-even effects as the fragments follow their decay chains, the consistent treatment of pairing may significantly enhance these staggering effects on the final yields. In the framework of this model, we find that odd-even effects in the charge distributions should be observed in the fragmentation of relatively light systems at very low excitation energies. Our results also suggest that the odd-even staggering may provide useful information on the nuclear state density.

  2. An electrostatic deceleration lens for highly charged ions

    International Nuclear Information System (INIS)

    The design and implementation of a purely electrostatic deceleration lens used to obtain beams of highly charged ions at very low energies is presented. The design of the lens is such that it can be used with parallel as well as diverging incoming beams and delivers a well focused low energy beam at the target. In addition, tuning of the final energy of the beam over a wide range (1 eV/q to several hundred eV/q, where q is the beam charge state) is possible without any change in hardware configuration. The deceleration lens was tested with Ar8+, extracted from an electron cyclotron resonance ion source, having an initial energy of 30 keV/q and final energies as low as 70 eV/q have been achieved.

  3. An electrostatic deceleration lens for highly charged ions.

    Science.gov (United States)

    Rajput, J; Roy, A; Kanjilal, D; Ahuja, R; Safvan, C P

    2010-04-01

    The design and implementation of a purely electrostatic deceleration lens used to obtain beams of highly charged ions at very low energies is presented. The design of the lens is such that it can be used with parallel as well as diverging incoming beams and delivers a well focused low energy beam at the target. In addition, tuning of the final energy of the beam over a wide range (1 eV/q to several hundred eV/q, where q is the beam charge state) is possible without any change in hardware configuration. The deceleration lens was tested with Ar(8+), extracted from an electron cyclotron resonance ion source, having an initial energy of 30 keV/q and final energies as low as 70 eV/q have been achieved. PMID:20441330

  4. Preparation of cold Mg+ion clouds for sympathetic cooling of highly charged ions at SPECTRAP

    International Nuclear Information System (INIS)

    The bound electrons in hydrogen-like or lithium-like heavy ions experience extremely strong electric and magnetic fields in the surrounding of the nucleus. Laser spectroscopy of the ground-state hyperfine splitting in the lead region provides a sensitive tool to test strong-field quantum electro dynamics (QED), especially in the magnetic sector. Previous measurements on hydrogen-like systems performed in an electron-beam ion trap (EBIT) or at the experimental storage ring (ESR) were experimentally limited in accuracy due to statistics, the large Doppler broadening and the ion energy. The full potential of the QED test can only be exploited if measurements for hydrogen- and lithium-like ions are performed with accuracy improved by 2-3 orders of magnitude. Therefore, the new Penning trap setup SPECTRAP - dedicated for laser spectroscopy on trapped and cooled highly charged ions - is currently commissioned at GSI Darmstadt. Heavy highly charged ions will be delivered to this trap by the HITRAP facility in the future. SPECTRAP is a cylindrical Penning trap with axial access for external ion injection and radial optical access mounted inside a cold-bore superconducting Helmholtz-type split-coil magnet. To reach the targeted accuracy in laser spectroscopy, an efficient and fast cooling process for the highly charged ions must be employed. This can be realized by sympathetic cooling with a cloud of laser-cooled light ions. Within this thesis work, a laser system and an ion source for the production of such a 24Mg+ ion cloud was developed and commissioned at SPECTRAP. An all-solid-state laser system for the generation of 279.6 nm light was designed and built. It consists of a fiber laser at 1118.5 nm followed by frequency quadrupling using two successive second-harmonic generation stages with actively stabilized ring resonators and nonlinear crystals. The laser system can deliver more than 15 mW of UV laser power under optimal conditions and requires little maintenance

  5. New development of laser ion source for highly charged ion beam production at Institute of Modern Physics (invited).

    Science.gov (United States)

    Zhao, H Y; Zhang, J J; Jin, Q Y; Liu, W; Wang, G C; Sun, L T; Zhang, X Z; Zhao, H W

    2016-02-01

    A laser ion source based on Nd:YAG laser has been being studied at the Institute of Modern Physics for the production of high intensity high charge state heavy ion beams in the past ten years, for possible applications both in a future accelerator complex and in heavy ion cancer therapy facilities. Based on the previous results for the production of multiple-charged ions from a wide range of heavy elements with a 3 J/8 ns Nd:YAG laser [Zhao et al., Rev. Sci. Instrum. 85, 02B910 (2014)], higher laser energy and intensity in the focal spot are necessary for the production of highly charged ions from the elements heavier than aluminum. Therefore, the laser ion source was upgraded with a new Nd:YAG laser, the maximum energy of which is 8 J and the pulse duration can be adjusted from 8 to 18 ns. Since then, the charge state distributions of ions from various elements generated by the 8 J Nd:YAG laser were investigated for different experimental conditions, such as laser energy, pulse duration, power density in the focal spot, and incidence angle. It was shown that the incidence angle is one of the most important parameters for the production of highly charged ions. The capability of producing highly charged ions from the elements lighter than silver was demonstrated with the incidence angle of 10° and laser power density of 8 × 10(13) W cm(-2) in the focal spot, which makes a laser ion source complementary to the superconducting electron cyclotron resonance ion source for the future accelerator complex especially in terms of the ion beam production from some refractory elements. Nevertheless, great efforts with regard to the extraction of intense ion beams, modification of the ion beam pulse duration, and reliability of the ion source still need to be made for practical applications. PMID:26931978

  6. New development of laser ion source for highly charged ion beam production at Institute of Modern Physics (invited)

    International Nuclear Information System (INIS)

    A laser ion source based on Nd:YAG laser has been being studied at the Institute of Modern Physics for the production of high intensity high charge state heavy ion beams in the past ten years, for possible applications both in a future accelerator complex and in heavy ion cancer therapy facilities. Based on the previous results for the production of multiple-charged ions from a wide range of heavy elements with a 3 J/8 ns Nd:YAG laser [Zhao et al., Rev. Sci. Instrum. 85, 02B910 (2014)], higher laser energy and intensity in the focal spot are necessary for the production of highly charged ions from the elements heavier than aluminum. Therefore, the laser ion source was upgraded with a new Nd:YAG laser, the maximum energy of which is 8 J and the pulse duration can be adjusted from 8 to 18 ns. Since then, the charge state distributions of ions from various elements generated by the 8 J Nd:YAG laser were investigated for different experimental conditions, such as laser energy, pulse duration, power density in the focal spot, and incidence angle. It was shown that the incidence angle is one of the most important parameters for the production of highly charged ions. The capability of producing highly charged ions from the elements lighter than silver was demonstrated with the incidence angle of 10° and laser power density of 8 × 1013 W cm−2 in the focal spot, which makes a laser ion source complementary to the superconducting electron cyclotron resonance ion source for the future accelerator complex especially in terms of the ion beam production from some refractory elements. Nevertheless, great efforts with regard to the extraction of intense ion beams, modification of the ion beam pulse duration, and reliability of the ion source still need to be made for practical applications

  7. New development of laser ion source for highly charged ion beam production at Institute of Modern Physics (invited)

    Science.gov (United States)

    Zhao, H. Y.; Zhang, J. J.; Jin, Q. Y.; Liu, W.; Wang, G. C.; Sun, L. T.; Zhang, X. Z.; Zhao, H. W.

    2016-02-01

    A laser ion source based on Nd:YAG laser has been being studied at the Institute of Modern Physics for the production of high intensity high charge state heavy ion beams in the past ten years, for possible applications both in a future accelerator complex and in heavy ion cancer therapy facilities. Based on the previous results for the production of multiple-charged ions from a wide range of heavy elements with a 3 J/8 ns Nd:YAG laser [Zhao et al., Rev. Sci. Instrum. 85, 02B910 (2014)], higher laser energy and intensity in the focal spot are necessary for the production of highly charged ions from the elements heavier than aluminum. Therefore, the laser ion source was upgraded with a new Nd:YAG laser, the maximum energy of which is 8 J and the pulse duration can be adjusted from 8 to 18 ns. Since then, the charge state distributions of ions from various elements generated by the 8 J Nd:YAG laser were investigated for different experimental conditions, such as laser energy, pulse duration, power density in the focal spot, and incidence angle. It was shown that the incidence angle is one of the most important parameters for the production of highly charged ions. The capability of producing highly charged ions from the elements lighter than silver was demonstrated with the incidence angle of 10° and laser power density of 8 × 1013 W cm-2 in the focal spot, which makes a laser ion source complementary to the superconducting electron cyclotron resonance ion source for the future accelerator complex especially in terms of the ion beam production from some refractory elements. Nevertheless, great efforts with regard to the extraction of intense ion beams, modification of the ion beam pulse duration, and reliability of the ion source still need to be made for practical applications.

  8. New development of laser ion source for highly charged ion beam production at Institute of Modern Physics (invited)

    Energy Technology Data Exchange (ETDEWEB)

    Zhao, H. Y., E-mail: zhaohy@impcas.ac.cn; Zhang, J. J.; Jin, Q. Y.; Sun, L. T.; Zhang, X. Z.; Zhao, H. W. [Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 730000 (China); Liu, W.; Wang, G. C. [Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 730000 (China); University of Chinese Academy of Sciences, Beijing 100049 (China)

    2016-02-15

    A laser ion source based on Nd:YAG laser has been being studied at the Institute of Modern Physics for the production of high intensity high charge state heavy ion beams in the past ten years, for possible applications both in a future accelerator complex and in heavy ion cancer therapy facilities. Based on the previous results for the production of multiple-charged ions from a wide range of heavy elements with a 3 J/8 ns Nd:YAG laser [Zhao et al., Rev. Sci. Instrum. 85, 02B910 (2014)], higher laser energy and intensity in the focal spot are necessary for the production of highly charged ions from the elements heavier than aluminum. Therefore, the laser ion source was upgraded with a new Nd:YAG laser, the maximum energy of which is 8 J and the pulse duration can be adjusted from 8 to 18 ns. Since then, the charge state distributions of ions from various elements generated by the 8 J Nd:YAG laser were investigated for different experimental conditions, such as laser energy, pulse duration, power density in the focal spot, and incidence angle. It was shown that the incidence angle is one of the most important parameters for the production of highly charged ions. The capability of producing highly charged ions from the elements lighter than silver was demonstrated with the incidence angle of 10° and laser power density of 8 × 10{sup 13} W cm{sup −2} in the focal spot, which makes a laser ion source complementary to the superconducting electron cyclotron resonance ion source for the future accelerator complex especially in terms of the ion beam production from some refractory elements. Nevertheless, great efforts with regard to the extraction of intense ion beams, modification of the ion beam pulse duration, and reliability of the ion source still need to be made for practical applications.

  9. Charge-state enhancement for radioactive beam post-acceleration

    International Nuclear Information System (INIS)

    A critical question for an ISOL-type radioactive-beam facility, such as that being discussed by the North American Isospin Laboratory Committee, is the efficiency and q/m of the ion source for the radioactive species. ISOLDE at CERN demonstrated that high efficiency is obtained for a wide variety of species in the 1+ charge state. These ion sources also generally have excellent transverse emittances and low energy spreads. One possibility is to use this proven technology plus an ionizer stage to increase the output of such sources to 2, 3, or 4+ with high efficiency. We are currently investigating technical options for such charge-state enhancement. There is a proposal by a Heidelberg/ISOLDE collaboration to build a open-quotes charge-state breederclose quotes as part of an experiment called REX-ISOLDE. This concept would deliver batches of radioactive ions with low duty cycle, optimized for relatively low-intensity secondary beams, on the order of 106/sec. We are independently doing simulations of an alternative approach, called the Electron-Beam Charge-State Amplifier (EBQA), which would yield DC beams with improved transverse emittance and would not have the intensity limitation of the batch transfer process. The cost and efficiency of the EBQA will have to be compared with those of a normally-conducting CW RFQ followed by ion stripping, as alternatives for the first stage of a secondary ion accelerator

  10. Energy dissipation of highly charged ions interacting with solid surfaces

    International Nuclear Information System (INIS)

    Motivated by the incomplete scientific description of the relaxation of highly charged ions in front of solid surfaces and their energy balance, this thesis describes an advanced complementary study of determining deposited fractions and re-emitted fractions of the potential energy of highly charged ions. On one side, a calorimetric measurement setup is used to determine the retained potential energy and on the other side, energy resolved electron spectroscopy is used for measuring the reemitted energy due to secondary electron emission. In order to study the mechanism of energy retention in detail, materials with different electronic structures are investigated: Cu, n-Si, p-Si and SiO2. In the case of calorimetry, a linear relationship between the deposited potential energy and the inner potential energy of the ions was determined. The total potential energy which stays in the solid remains almost constant at about (80 ± 10) %. Comparing the results of the Cu, n-Si and p-Si targets, no significant difference could be shown. Therefore we conclude that the difference in energy deposition between copper, n-doped Si and p-doped Si is below 10 %, which is significantly lower than using SiO2 targets. For this purpose, electron spectroscopy provides a complementary result. For Cu and Si surfaces, an almost linear increase of the re-emitted energy with increasing potential energy of the ion up to Ar7+ was also observed. The ratio of the re-emitted energy is about (10 ± 5) % of the total potential energy of the incoming ion, almost independent of the ion charge state. In contrast, an almost vanishing electron emission was observed for SiO2 and for charge states below q=7. For Ar8+ and Ar9+, the electron emission increased due to the contribution of the projectile LMM Auger electrons and the re-emitted energy amounts up to 20 % for Cu and Si and around 10 % for SiO2. These results are in good agreement with the calorimetric values. In addition, the experimental results

  11. Scintillation light produced by low-energy beams of highly-charged ions

    OpenAIRE

    M. Vogel; Winters, D.F.A.; Ernst, H.; H. Zimmermann; Kester, O.

    2007-01-01

    Measurements have been performed of scintillation light intensities emitted from various inorganic scintillators irradiated with low-energy beams of highly-charged ions from an electron beam ion source (EBIS) and an electron cyclotron resonance ion source (ECRIS). Beams of xenon ions Xe$^{q+}$ with various charge states between $q$=2 and $q$=18 have been used at energies between 5 keV and 17.5 keV per charge generated by the ECRIS. The intensity of the beam was typically varied between 1 and ...

  12. EXPERIMENTAL INVESTIGATIONS OF ION CHARGE DISTRIBUTIONS, EFFECTIVE ELECTRON DENSITIES, AND ELECTRON-ION CLOUD OVERLAP IN ELECTRON BEAM ION TRAP PLASMA USING EXTREME-ULTRAVIOLET SPECTROSCOPY

    International Nuclear Information System (INIS)

    Spectra in the extreme ultraviolet range from 107 to 353 A emitted from Fe ions in various ionization stages have been observed at the Heidelberg electron beam ion trap (EBIT) with a flat-field grating spectrometer. A series of transition lines and their intensities have been analyzed and compared with collisional-radiative simulations. The present collisional-radiative model reproduces well the relative line intensities and facilitates line identification of ions produced in the EBIT. The polarization effect on the line intensities resulting from nonthermal unidirectional electron impact was explored and found to be significant (up to 24%) for a few transition lines. Based upon the observed line intensities, relative charge state distributions (CSD) of ions were determined, which peaked at Fe23+ tailing toward lower charge states. Another simulation on ion charge distributions including the ionization and electron capture processes generated CSDs which are in general agreement with the measurements. By observing intensity ratios of specific lines from levels collisionally populated directly from the ground state and those starting from the metastable levels of Fe XXI, Fe X and other ionic states, the effective electron densities were extracted and found to depend on the ionic charge. Furthermore, it was found that the overlap of the ion cloud with the electron beam estimated from the effective electron densities strongly depends on the charge state of the ion considered, i.e. under the same EBIT conditions, higher charge ions show less expansion in the radial direction.

  13. Photoionization of multiply charged ions at the advanced light source

    OpenAIRE

    Schlachter, A. S.; Kilcoyne, A. L. D.; Aguilar, A.; Gharaibeh, M. F.; Emmons, E. D.; Scully., S. W. J.; Phaneuf, R A; Muller, A.; Schippers, S.; I. Alvarez; Cisneros, C.; Hinojosa, G.; McLaughlin, B. M.

    2004-01-01

    Photoionization of multiply charged ions is studied using the merged-beams technique at the Advanced Light Source. Absolute photoionization cross sections have been measured for a variety of ions along both isoelectronic and isonuclear sequences.

  14. Optimal foil material and thickness for the charge stripping of heavy ions of around 100 MeV

    International Nuclear Information System (INIS)

    In order to seek an optimal charge stripping material and its thickness for the charge stripping of heavy ions of around 100 MeV, the transmission of highly charged ions after passage through charge stripping foils has been measured using 95 MeV Cl ions. Tested foils are Be and C foils of various thicknesses. As a result, Be foils with several tens of μg/cm2 are most efficient for the obtainment of highly charged ions whose charge states are higher than the most probable charge state. On the other hand, for the use of ions with the most probable charge state, there is no noticeable difference between the use of C and Be foils provided that their thicknesses are a few tends of μg/cm2. (orig.)

  15. Highly charged ions impinging on a stepped metal surface under grazing incidence

    NARCIS (Netherlands)

    Robin, A; Niemann, D; Stolterfoht, N; Heiland, W

    2003-01-01

    We report on energy loss measurements and charge state distributions for 60 keV N6+ and 75 keV N5+ ions scattered off a Pt(110)(1x2) single crystal surface. In particular, the influence of surface steps on the energy loss and the outgoing charge states is discussed. The scattering angle and the angl

  16. A trapped ion source with improved ionizing efficiency for the production of multiply charged ions

    International Nuclear Information System (INIS)

    An ultrahigh vacuum 'trapped ion source' has been developed following closely Redhead's basic design. Positive ions have been trapped within the space charge of a magnetically confined electron beam with potential barriers at either end of the ionization region, resulting in the production of multiply charged ions. These highly stripped ions are formed by the successive collisions with low energy (0 mass spectrometer. The results obtained in the production of multiply charged ions of Au are presented. (auth.)

  17. Measurements of Ion Selective Containment on the RF Charge Breeder Device BRIC

    CERN Document Server

    Variale, Vincenzo; Batazova, Marina; Boggia, Antonio; Clauser, Tarcisio; Kuznetsov, Gennady I; Rainò, Antonio; Shiyankov, Sergey; Skarbo, Boris A; Valentino, Vincenzo; Verrone, Grazia

    2005-01-01

    The "charge state breeder" BRIC (BReeding Ion Charge) is based on an EBIS source and it is designed to accept Radioactive Ion Beam (RIB) with charge +1, in a slow injection mode, to increase their charge state up to +n. BRIC has been developed at the INFN section of Bari (Italy) during these last 3 years with very limited funds. Now, it has been assembled at the LNL (Italy) where are in progress the first tests as stand alone source. The new feature of BRIC, with respect to the classical EBIS, is given by the insertion, in the ion drift chamber, of a Radio Frequency (RF) Quadrupole aiming to filtering the unwanted elements and then making a more efficient containment of the wanted ions. In this contribution, the measurements of the selective effect on the ion charge state containement of the RF quadrupole field, applied on the ion chamber, will be reported and discussed. The ion charge state analisys of the ions trapped in BRIC seem confirm, as foreseen by simulation results carried out previously, that the s...

  18. Electron emission and defect formation in the interaction of slow, highly charged ions with diamond surfaces

    OpenAIRE

    Sideras-Haddad, E.; Shrivastava, S; Rebuli, D.B.; Persaud, A.; Schneider, D. H.; Schenkel, T.

    2008-01-01

    We report on electron emission and defect formation in the interaction between slow (v~;0.3 vBohr) highly charged ions (SHCI) with insulating (type IIa) and semiconducting (type IIb) diamonds. Electron emission induced by 31Pq+ (q=5 to 13), and 136Xeq+ (q=34 to 44) with kinetic energies of 9 kVxq increase linearly with the ion charge states, reaching over 100 electrons per ion for high xenon charge states without surface passivation of the diamond with hydrogen. Yields from both diamond ...

  19. Tuning Charge Transfer in Ion-Surface Collisions at Hyperthermal Energies.

    Science.gov (United States)

    Yao, Yunxi; Giapis, Konstantinos P

    2016-05-18

    Charge exchange in ion-surface collisions may be influenced by surface adsorbates to alter the charge state of the scattered projectiles. We show here that the positive-ion yield, observed during ion scattering on metal surfaces at low incident energies, is greatly enhanced by adsorbing electronegative species onto the surface. Specifically, when beams of N(+) and O(+) ions are scattered off of clean Au surfaces at hyperthermal energies, no positive ions are observed exiting. Partial adsorption of F atoms on the Au surface, however, leads to the appearance of positively charged primary ions scattering off of Au, a direct result of the increase in the Au work function. The inelastic energy losses for positive-ion exits are slightly larger than the corresponding ionization energies of the respective N and O atoms, which suggest that the detected positive ions are formed by surface reionization during the hard collision event. PMID:26879471

  20. Role of Ion-Surface Interaction at the Entry Surface on the Energy Loss of Highly Charged Slow Ions in Solids

    OpenAIRE

    Tapan Nandi

    2011-01-01

    Evidence is obtained from the data of an earlier measurement that the effect of ion-surface interaction on the stopping power of highly charged slow ions is not at all tiny rather remarkably large, even it supersedes the bulk stopping power. The stopping power due to the surface interactions is directly proportional to the charge state of incident ions.

  1. Cooling of highly charged ions in a Penning trap

    Energy Technology Data Exchange (ETDEWEB)

    Gruber, L

    2000-03-31

    Highly charged ions are extracted from an electron beam ion trap and guided to Retrap, a cryogenic Penning trap, where they are merged with laser cooled Be{sup +} ions. The Be{sup +} ions act as a coolant for the hot highly charged ions and their temperature is dropped by about 8 orders of magnitude in a few seconds. Such cold highly charged ions form a strongly coupled nonneutral plasma exhibiting, under such conditions, the aggregation of clusters and crystals. Given the right mixture, these plasmas can be studied as analogues of high density plasmas like white dwarf interiors, and potentially can lead to the development of cold highly charged ion beams for applications in nanotechnology. Due to the virtually non existent Doppler broadening, spectroscopy on highly charged ions can be performed to an unprecedented precision. The density and the temperature of the Be{sup +} plasma were measured and highly charged ions were sympathetically cooled to similar temperatures. Molecular dynamics simulations confirmed the shape, temperature and density of the highly charged ions. Ordered structures were observed in the simulations.

  2. High-precision atomic clocks with highly charged ions: nuclear spin-zero $f^{12}$-shell ions

    OpenAIRE

    Dzuba, V. A.; Derevianko, A; Flambaum, V. V.

    2012-01-01

    Optical atomic clocks using highly-charged ions hold an intriguing promise of metrology at the 19th significant figure. Here we study transitions within the $4f^{12}$ ground-state electronic configuration of highly charged ions. We consider isotopes lacking hyperfine structure and show that the detrimental effects of coupling of electronic quadrupole moments to gradients of trapping electric field can be effectively reduced by using specially chosen virtual clock transitions. The estimated sy...

  3. Multiply charged ion sources for photon-ion crossed beam experiments

    International Nuclear Information System (INIS)

    The intense beams of synchrotron radiation which will be available from dedicated storage rings such as the x-ray and vuv rings at the National Synchrotron Light Source allow one to contemplate experimental arrangements which can be used to investigate photon-ion interactions in the x-ray and vuv ranges. Studies of multiple charged ions of charge greater than two and their interactions with photons are of great interest because of the general lack of experimental information about the properties of ground and highly excited states of such ions and the important role some multiply charged ions play in astrophysical and laboratory plasmas. Experimental arrangements which would allow the use of photons as probes of such systems would be invaluable in these studies and would help stimulate research in a thus far untouched but increasingly important area of atomic physics. Specific experimental arrangements will depend on the aspects of the interaction being studied, but in general the experiments will be technically difficult and by necessity will involve crossed ion-photon beams with concomitant small interaction rates

  4. Aerosol charge state characterisation using an ELPI

    Energy Technology Data Exchange (ETDEWEB)

    Matthews, J C; Wright, M D; Henshaw, D L [University of Bristol (United Kingdom); Biddiscombe, M F; Usmani, O S, E-mail: j.c.matthews@bristol.ac.uk [NHLI, Imperial College London and Royal Brompton Hospital (United Kingdom)

    2011-06-23

    A new technique has been developed to measure the size distribution and charge state of highly charged aerosols using an Electrical Low Pressure Impactor (ELPI). The internal charger was switched alternately on and off and the time between stable charge states found to be {approx} 10 s. The size distribution of aerosols was found when the charger was on, from which the charge distribution can be estimated when the charger is off using the current at each impactor stage. This method was tested in background conditions, when a candle was burning and when a negative air ioniser was used. The ELPI electrometers were not sensitive enough to accurately measure the charge state on background and candle air, but gave a value for air charged by an ioniser. Comparing results from the ELPI with other techniques showed inaccuracies in this method that need to be addressed before further use of this technique.

  5. Aerosol charge state characterisation using an ELPI

    Science.gov (United States)

    Matthews, J. C.; Wright, M. D.; Biddiscombe, M. F.; Usmani, O. S.; Henshaw, D. L.

    2011-06-01

    A new technique has been developed to measure the size distribution and charge state of highly charged aerosols using an Electrical Low Pressure Impactor (ELPI). The internal charger was switched alternately on and off and the time between stable charge states found to be ~ 10 s. The size distribution of aerosols was found when the charger was on, from which the charge distribution can be estimated when the charger is off using the current at each impactor stage. This method was tested in background conditions, when a candle was burning and when a negative air ioniser was used. The ELPI electrometers were not sensitive enough to accurately measure the charge state on background and candle air, but gave a value for air charged by an ioniser. Comparing results from the ELPI with other techniques showed inaccuracies in this method that need to be addressed before further use of this technique.

  6. Ion momentum and energy transfer rates for charge exchange collisions

    Science.gov (United States)

    Horwitz, J.; Banks, P. M.

    1973-01-01

    The rates of momentum and energy transfer have been obtained for charge exchange collisions between ion and neutral gases having arbitrary Maxwellian temperatures and bulk transport velocities. The results are directly applicable to the F-region of the ionosphere where 0+ - 0 charge is the dominant mechanism affecting ion momentum and energy transfer.

  7. Problems with Accurate Atomic Lfetime Measurements of Multiply Charged Ions

    Energy Technology Data Exchange (ETDEWEB)

    Trabert, E

    2009-02-19

    A number of recent atomic lifetime measurements on multiply charged ions have reported uncertainties lower than 1%. Such a level of accuracy challenges theory, which is a good thing. However, a few lessons learned from earlier precision lifetime measurements on atoms and singly charged ions suggest to remain cautious about the systematic errors of experimental techniques.

  8. Maximizing Ion Current by Space Charge Neutralization using Negative Ions and Dust Particles

    International Nuclear Information System (INIS)

    Ion current extracted from an ion source (ion thruster) can be increased above the Child-Langmuir limit if the ion space charge is neutralized. Similarly, the limiting kinetic energy density of the plasma flow in a Hall thruster might be exceeded if additional mechanisms of space charge neutralization are introduced. Space charge neutralization with high-mass negative ions or negatively charged dust particles seems, in principle, promising for the development of a high current or high energy density source of positive light ions. Several space charge neutralization schemes that employ heavy negatively charged particles are considered. It is shown that the proposed neutralization schemes can lead, at best, only to a moderate but nonetheless possibly important increase of the ion current in the ion thruster and the thrust density in the Hall thruster

  9. Ion and water transport in charge-modified graphene nanopores

    CERN Document Server

    Qiu, Yinghua; Chen, Weiyu; Si, Wei; Tan, Qiyan; Chen, Yunfei

    2016-01-01

    Porous graphene has high mechanical strength and atomic layer thickness, which make it a promising material for material separation and biomolecule sensing. Electrostatic interactions between charges in aqueous solution are a kind of strong long-range interaction which may have great influence on the fluid transport through nanopores. Here, molecular dynamics simulations were conducted to investigate ion and water transport through a 1.05-nm-in-diameter monolayer graphene nanopore with its edge charge-modified. From the results, it is found that the nanopores are selective to counterions when they are charged. As the charge amount increases, the total ionic currents show an increase-decrease profile while the co-ion currents monotonously decrease. The co-ions rejection can reach 75% and 90% when the nanopores are negatively and positively charged, respectively. Cl ions current increases and reaches a plateau, and Na+ current decreases with the charge amount in the systems where they act as counterions. Beside...

  10. In-situ Studies of Highly Charged Ions at the LLNL EBIT

    Energy Technology Data Exchange (ETDEWEB)

    Beiersdorfer, P

    2001-08-16

    The properties of highly charged ions and their interaction with electrons and atoms is being studied in-situ at the LLNL electron beam ion traps, EBIT-II and SuperEBIT. Spectroscopic measurements provide data on electron-ion and ion-atom interactions as well as accurate transition energies of lines relevant for understanding QED, nuclear magnetization, and the effects of relativity on complex, state-of-the-art atomic calculations.

  11. Heavy-ion radiography applied to charged particle radiotherapy

    International Nuclear Information System (INIS)

    The objectives of the heavy-ion radiography research program applied to the clinical cancer research program of charged particle radiotherapy have a twofold purpose: (1) to explore the manner in which heavy-ion radiography and CT reconstruction can provide improved tumor localization, treatment planning, and beam delivery for radiotherapy with accelerated heavy charged particles; and (2) to explore the usefulness of heavy-ion radiography in detecting, localizing, and sizing soft tissue cancers in the human body. The techniques and procedures developed for heavy-ion radiography should prove successful in support of charged particle radiotherapy

  12. Experimental results on charge fluctuations in heavy-ion collisions

    CERN Document Server

    Mishra, D K; Netrakanti, P K; Pant, L M; Mohanty, A K

    2016-01-01

    We present a subset of experimental results on charge fluctuation from the heavy-ion collisions to search for phase transition and location of critical point in the QCD phase diagram. Measurements from the heavy-ion experiments at the SPS and RHIC energies observe that total charge fluctuations increase from central to peripheral collisions. The net-charge fluctuations in terms of dynamical fluctuation measure $\

  13. Dynamic battery cell model and state of charge estimation

    Science.gov (United States)

    Wijewardana, S.; Vepa, R.; Shaheed, M. H.

    2016-03-01

    Mathematical modelling and the dynamic simulation of battery storage systems can be challenging and demanding due to the nonlinear nature of the battery chemistry. This paper introduces a new dynamic battery model, with application to state of charge estimation, considering all possible aspects of environmental conditions and variables. The aim of this paper is to present a suitable convenient, generic dynamic representation of rechargeable battery dynamics that can be used to model any Lithium-ion rechargeable battery. The proposed representation is used to develop a dynamic model considering the thermal balance of heat generation mechanism of the battery cell and the ambient temperature effect including other variables such as storage effects, cyclic charging, battery internal resistance, state of charge etc. The results of the simulations have been used to study the characteristics of a Lithium-ion battery and the proposed battery model is shown to produce responses within 98% of known experimental measurements.

  14. Ion Transport through Diffusion Layer Controlled by Charge Mosaic Membrane

    Directory of Open Access Journals (Sweden)

    Akira Yamauchi

    2012-01-01

    Full Text Available The kinetic transport behaviors in near interface of the membranes were studied using commercial anion and cation exchange membrane and charge mosaic membrane. Current-voltage curve gave the limiting current density that indicates the ceiling of conventional flux. From chronopotentiometry above the limiting current density, the transition time was estimated. The thickness of boundary layer was derived with conjunction with the conventional limiting current density and the transition time from steady state flux. On the other hand, the charge mosaic membrane was introduced in order to examine the ion transport on the membrane surface in detail. The concentration profile was discussed by the kinetic transport number with regard to the water dissociation (splitting on the membrane surface.

  15. Two-photon processes in highly charged ions

    International Nuclear Information System (INIS)

    Two-photon processes are atomic processes in which an atom interacts simultaneously with two photons. Such processes describe a wide range of phenomena, such as two-photon decay and elastic or inelastic scattering of photons. In recent years two-photon processes involving highly charged heavy ions have become an active area of research. Such studies do not only consider the total transition or scattering rates but also their angular and polarization dependence. To support such examinations in this thesis I present a theoretical framework to describe these properties in all two-photon processes with bound initial and final states and involving heavy H-like or He-like ions. I demonstrate how this framework can be used in some detailed studies of different two-photon processes. Specifically a detailed analysis of two-photon decay of H-like and He-like ions in strong external electromagnetic fields shows the importance of considering the effect of such fields for the physics of such systems. Furthermore I studied the elastic Rayleigh as well as inelastic Raman scattering by heavy H-like ions. I found a number of previously unobserved phenomena in the angular and polarization dependence of the scattering cross-sections that do not only allow to study interesting details of the electronic structure of the ion but might also be useful for the measurement of weak physical effects in such systems.

  16. Two-photon processes in highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Jahrsetz, Thorsten

    2015-03-05

    Two-photon processes are atomic processes in which an atom interacts simultaneously with two photons. Such processes describe a wide range of phenomena, such as two-photon decay and elastic or inelastic scattering of photons. In recent years two-photon processes involving highly charged heavy ions have become an active area of research. Such studies do not only consider the total transition or scattering rates but also their angular and polarization dependence. To support such examinations in this thesis I present a theoretical framework to describe these properties in all two-photon processes with bound initial and final states and involving heavy H-like or He-like ions. I demonstrate how this framework can be used in some detailed studies of different two-photon processes. Specifically a detailed analysis of two-photon decay of H-like and He-like ions in strong external electromagnetic fields shows the importance of considering the effect of such fields for the physics of such systems. Furthermore I studied the elastic Rayleigh as well as inelastic Raman scattering by heavy H-like ions. I found a number of previously unobserved phenomena in the angular and polarization dependence of the scattering cross-sections that do not only allow to study interesting details of the electronic structure of the ion but might also be useful for the measurement of weak physical effects in such systems.

  17. Dissociation of OCS by high energy highly charged ion impact

    International Nuclear Information System (INIS)

    OCS is an important molecule with immense biological, chemical and astrophysical significance. Various dissociation channels of OCSq+ (where q = 2 to 4), formed in the interaction of 5 MeV u-1 Si12+ ion beam with neutral OCS, have been studied using recoil-ion momentum spectroscopy. The concerted and/or sequential nature of dissociation is inferred from the shape and slope of the coincidence islands in the 2D coincidence map. It is observed that the C+ + S+ + O channel results from concerted as well as sequential decay of OCS2+. However the other channels originate purely from the concerted process in which the two terminal fragments (oxygen and sulphur) fly back to back and the central carbon fragment is left with negligible momentum. The kinetic energy release (KER) distributions for all the fragmentation channels arising from the dissociation of OCSq+ (where q = 2 to 4) have been measured and compared with the available data in the literature. It is observed that the KER values for complete Coulomb fragmentation channels are much smaller than those of incomplete Coulomb fragmentation cases and the KER increases with the increasing charge states of the parent molecular ions. From the momentum correlation map, we estimated the geometry of the precursor molecular ion undergoing three-body dissociation and inferred that bent dissociative states are involved in most of the fragmentation channels of OCSq+. (authors)

  18. Study on High Intensity High Charge State Lead Ion Beam Production and Optimize%强流高电荷态Pb离子束的产生与优化研究

    Institute of Scientific and Technical Information of China (English)

    何伟; 李锦钰; 赵环昱; 曹云; 孙良亭; 赵红卫; 张子民

    2005-01-01

    随着原子物理及表面物理研究的发展,高电荷态金属离子束的需求日益增多.近来,在中国科学院近代物理研究所14.5GHz LECR3离子源实验平台上,以炉子法产生的铅离子束作为研究对象,进行了一系列ECR离子源关键参数(如:磁场、炉子功率、掺气等)影响高电荷态铅离子束产额的实验研究,在此基础上,调整优化了LECR3离子源的状态参数,从而获得了强流高电荷态铅离子束18etA 207pb30+和6.7eμA207pb37+.%High charge state metal ion beam is quite effective and essential for new investigations on atomic physics and surface physics. Recently, The high intensity high charge state lead ion beams have been produced with IMP 14.5GHz LECR3, we investigated experimentally influences of some key parameters,such as magnetic field, electrical power on oven, gas mixing etc., on lead ion beam production. Through optimization of the ion source conditions, stable 207Pb30+ beam of 18eμA and 207Pb37+ beam of 6.7eμA have been obtained with oven method at 20kV extraction voltage.

  19. KLL Dielectronic Recombination of Highly Charged Sulfur and Silicon Ions

    OpenAIRE

    Ali, Safdar

    2014-01-01

    Dielectronic recombination measurements for highly charged ions were performed at the Stockholm refrigerated electron beam ion trap. We have obtained KLL DR resonance strengths for highly charged H- and He-like sulfur and silicon ions. The experimental results are compared with the theoretical data obtained from GRASP II code. Both the experimental and calculated results agree well within the experimental error bars. Moreover, the dielectronic recombination resonance strengths are used to obt...

  20. Capture and isolation of highly-charged ions in a unitary Penning trap

    CERN Document Server

    Brewer, Samuel M; Tan, Joseph N

    2013-01-01

    We recently used a compact Penning trap to capture and isolate highly-charged ions extracted from an electron beam ion trap (EBIT) at the National Institute of Standards and Technology (NIST). Isolated charge states of highly-stripped argon and neon ions with total charge $Q \\geq 10$, extracted at energies of up to $4\\times 10^3\\,Q$ eV, are captured in a trap with well depths of $\\,\\approx (4\\, {\\rm to}\\, 12)\\,Q$ eV. Here we discuss in detail the process to optimize velocity-tuning, capture, and storage of highly-charged ions in a unitary Penning trap designed to provide easy radial access for atomic or laser beams in charge exchange or spectroscopic experiments, such as those of interest for proposed studies of one-electron ions in Rydberg states or optical transitions of metastable states in multiply-charged ions. Under near-optimal conditions, ions captured and isolated in such rare-earth Penning traps can be characterized by an initial energy distribution that is $\\approx$ 60 times narrower than typically...

  1. Capture and isolation of highly-charged ions in a unitary Penning trap

    OpenAIRE

    Brewer, Samuel M.; Nicholas D. Guise; Tan, Joseph N

    2013-01-01

    We recently used a compact Penning trap to capture and isolate highly-charged ions extracted from an electron beam ion trap (EBIT) at the National Institute of Standards and Technology (NIST). Isolated charge states of highly-stripped argon and neon ions with total charge $Q \\geq 10$, extracted at energies of up to $4\\times 10^3\\,Q$ eV, are captured in a trap with well depths of $\\,\\approx (4\\, {\\rm to}\\, 12)\\,Q$ eV. Here we discuss in detail the process to optimize velocity-tuning, capture, ...

  2. Dynamics of multiply charged ions in intense laser fields

    CERN Document Server

    Hu, S X

    2000-01-01

    We numerically investigate the dynamics of multiply charged hydrogenic ions in near-optical linearly polarized laser fields with intensities of order 10^16 to 10^17 W/cm^2. Depending on the charge state Z of the ion the relation of strength between laser field and ionic core changes. We find around Z=12 typical multiphoton dynamics and for Z=3 tunneling behaviour, however with clear relativistic signatures. In first order in v/c the magnetic field component of the laser field induces a Z-dependent drift in the laser propagation direction and a substantial Z-dependent angular momentum with repect to the ionic core. While spin oscillations occur already in first order in v/c as described by the Pauli equation, spin induced forces via spin orbit coupling only appear in the parameter regime where (v/c)^2 corrections are significant. In this regime for Z=12 ions we show strong splittings of resonant spectral lines due to spin-orbit coupling and substantial corrections to the conventional Stark shift due to the rel...

  3. An Ion Switch Regulates Fusion of Charged Membranes

    Science.gov (United States)

    Siepi, Evgenios; Lutz, Silke; Meyer, Sylke; Panzner, Steffen

    2011-01-01

    Here we identify the recruitment of solvent ions to lipid membranes as the dominant regulator of lipid phase behavior. Our data demonstrate that binding of counterions to charged lipids promotes the formation of lamellar membranes, whereas their absence can induce fusion. The mechanism applies to anionic and cationic liposomes, as well as the recently introduced amphoteric liposomes. In the latter, an additional pH-dependent lipid salt formation between anionic and cationic lipids must occur, as indicated by the depletion of membrane-bound ions in a zone around pH 5. Amphoteric liposomes fuse under these conditions but form lamellar structures at both lower and higher pH values. The integration of these observations into the classic lipid shape theory yielded a quantitative link between lipid and solvent composition and the physical state of the lipid assembly. The key parameter of the new model, κ(pH), describes the membrane phase behavior of charged membranes in response to their ion loading in a quantitative way. PMID:21575575

  4. Fundamental processes determining the highly charged ion production in ECR ion sources

    International Nuclear Information System (INIS)

    The ion confinement and loss conditions in the open magnetic traps have been analyzed in this article. In EGRIS the the ions are confined in the negative potential well. The simultaneous application of ion cooling and pulse regime is proposed for pulse injection of highly charged ions in heavy ion accelerators and storage rings. 14 refs.; 3 figs

  5. Fragmentation of molecules under charge-changing collisions of a few MeV heavy ions

    International Nuclear Information System (INIS)

    We investigated molecular fragmentation of CO and C2H2 molecules by impact of various fast heavy ions. Fragment ions produced in electron capture and loss collisions of projectile ions were measured in coincidence with final projectile charge states. Data acquisition using position sensitive detection system allows us to obtain 3D momentum imaging of fragment ions and kinetic energy release (KER) in various charge-changing collisions. It was found that the KER spectra show strong dependence on the type of charge-changing collisions. This may be caused by the difference of impact parameters associated with individual charge-changing collisions. Moreover we revealed the different fragmentation pathway between ion impacts and photoionization

  6. Spatial distribution of ion charges in fast, partially stripped clusters traversing solid targets

    CERN Document Server

    Miskovic, Z L; Goodman, F O; Wang, Y N

    2002-01-01

    Joint statistical description of the distribution of ion charge states and the spatial structure of a cluster, made of heavy ions, allows a self-consistent generalization of the Brandt-Kitagawa variational theory, including dynamically-screened inter-ionic interactions, in a form of a non-linear integral equation. Solution of such an equation for fast clusters passing very thin foils shows the familiar reduction of charge per ion, compared to the charge on an isotactic ion, which is rather non-homogeneously distributed throughout the volume of the cluster. As a consequence, the distribution of individual ion charges in the cluster exhibits large dispersion around an average value, which drops with the increasing cluster size.

  7. Spatial distribution of ion charges in fast, partially stripped clusters traversing solid targets

    International Nuclear Information System (INIS)

    Joint statistical description of the distribution of ion charge states and the spatial structure of a cluster, made of heavy ions, allows a self-consistent generalization of the Brandt-Kitagawa variational theory, including dynamically-screened inter-ionic interactions, in a form of a non-linear integral equation. Solution of such an equation for fast clusters passing very thin foils shows the familiar reduction of charge per ion, compared to the charge on an isotactic ion, which is rather non-homogeneously distributed throughout the volume of the cluster. As a consequence, the distribution of individual ion charges in the cluster exhibits large dispersion around an average value, which drops with the increasing cluster size

  8. Average charge of superheavy recoil ion in helium gas

    Energy Technology Data Exchange (ETDEWEB)

    Kaji, D.; Morita, K.; Morimoto, K.; Haba, H. [RIKEN, Wako, Saitama (Japan). Nishina Center for Accelerator Based Science; Kudo, H. [Niigata Univ. (Japan). Dept. of Chemistry

    2011-07-01

    The average equilibrium charges q{sub ave} of heavy recoil ions moving in helium gas were measured by a gasfilled recoil ion separator (GARIS). A new empirical formula to calculate q{sub ave} for superheavy recoil ions with a low velocity was derived. This formula was applicable to the search for a superheavy nuclide of {sup 266}Bh. (orig.)

  9. Average charge of superheavy recoil ion in helium gas

    International Nuclear Information System (INIS)

    The average equilibrium charges qave of heavy recoil ions moving in helium gas were measured by a gasfilled recoil ion separator (GARIS). A new empirical formula to calculate qave for superheavy recoil ions with a low velocity was derived. This formula was applicable to the search for a superheavy nuclide of 266Bh. (orig.)

  10. Optimization of electron-cyclotron-resonance charge-breeder ions : Final CRADA Report.

    Energy Technology Data Exchange (ETDEWEB)

    Pardo, R.; Physics; Far-Tech, Inc.

    2009-10-09

    Measurements of 1+ beam properties and associated performance of ECR Charge Breeder source determined by total efficiency measurement and charge state distributions from the ECR Charge Breeder. These results were communicated to Far-Tech personnel who used them to benchmark the newly developed programs that model ion capture and charge breeding in the ECR Charge Breeder Source. Providing the basic data described above and in the discussion below to Far-Tech allowed them to improve and refine their calculational tools for ECR ion sources. These new tools will be offered for sale to industry and will also provide important guidance to other research labs developing Charge Breeding ion sources for radioactive beam physics research.

  11. Highly charged ions trapping for lifetime measurements; Piegeage d'ions tres charges pour la mesure de duree de vie d'etats metastables

    Energy Technology Data Exchange (ETDEWEB)

    Attia, D

    2007-10-15

    A new experimental setup dedicated to highly charged ion trapping is presented in this work. The final goal is to perform lifetime measurement of metastable states produced by our ECR (Electron Cyclotron Resonance) ion source. Lifetimes to be measured are in the range of a few ms and more. We have measured the lifetimes of the M1 transitions of the metastable states of Ar{sup 9+}, Ar{sup 13+} and Ar{sup 14+}. These measurements are useful to test the N-body problem in the relativistic range. The trap we have built, was designed a few years ago at the Weizman Institute in Israel, it allows ions with an energy of several keV to be trapped for lifetimes of about 1 second. This trap was originally designed to study the dynamics of excited molecules. We have shown for the first time how the trap operates and that it can operate with highly charged ions. We have studied the beam dynamics of highly charged ions and the trap has been tested with various species of ions and different charge states: from O{sup +} to O{sup 6+}, from Ar{sup 8+} to Ar{sup 13+}, and from Kr{sup 13+} to Kr{sup 20+}.

  12. Electron cyclotron resonance charge breeder ion source simulation by MCBC and GEM

    International Nuclear Information System (INIS)

    Numerical simulation results by the GEM and MCBC codes are presented, along with a comparison with experiments for beam capture dynamics and parameter studies of charge state distribution (CSD) of electron cyclotron resonance charge breeder ion sources. First, steady state plasma profiles are presented by GEM with respect to key experimental parameters such as rf power and gas pressure. As rf power increases, electron density increases by a small amount and electron energy by a large amount. The central electrostatic potential dip also increased. Next, MCBC is used to trace injected beam ions to obtain beam capture profiles. Using the captured ion profiles, GEM obtains a CSD of beam ions. As backscattering can be significant, capturing the ions near the center of the device enhances the CSD. The effect of rf power on the beam CSD is mainly due to different steady states plasmas. Example cases are presented assuming that the beam ions are small enough not to affect the plasma

  13. Studies of highly charged ions with EBIT and Super-EBIT

    International Nuclear Information System (INIS)

    The LLNL electron beam ion traps provide cold highly charged ions up to bare U. These machines have provided a wealth of atomic physics data using a compact, relatively inexpensive, device. The physics program has studied electron-ion collisions, QED, ion-surface interactions, and plasmas physics among many other topics. The prospects for the study of the highest charge states in the highest Z ions led to the beam energy upgrade of the first EBIT into Super-EBIT. The desire to use ions as a research probe in themselves led to an ion extraction program on EBIT-2. Finally, a Penning trap (referred to as the RETRAP) has been constructed to catch extracted ions where they can be further cooled and studied. Results of several experiments at the LLNL EBIT facility are described. The program's capabilities are discussed

  14. Light-induced charging effects in microscopic ion traps

    International Nuclear Information System (INIS)

    Full text: Microfabricated ion traps are discussed as one of the most promising candidates for a quantum mechanical computer. By bringing the electrodes close to the ions a rich selection of trapping potentials can be created and many traps can, in principle, be operated in parallel. However, the proximity of the electrodes and other surfaces poses strong constraints on the materials used. In particular, near-by glass surfaces that may be used for high-finesse cavities around the ions or for light collection represent a challenge, since the dielectric surfaces may charge up and perturb the trapping potential. By bringing a glass substrate close to a surface ion trap, the charging can be studied in a controlled manner. Two distinct mechanisms of charging have been observed, both being light-induced with different wavelength dependence. The results allow an estimate of the rate of charge production and may be prove useful for the design of new integrated microscopic ion traps. (author)

  15. Multiply charged neon cluster ions: critical size and Coulomb explosion

    International Nuclear Information System (INIS)

    Full text: Multiply charged neon cluster ions are formed upon electron impact ionization of large neutral clusters and analyzed utilizing a two sector field mass spectrometer applying techniques developed recently. The critical size for doubly charged neon cluster ions is determined experimentally with isotopically pure 20Ne to be 287. In spectra of natural neon, the presence of doubly charged clusters can be observed as an increase of the ion yield at the same cluster size confirming the above result. This method allows in addition an approximate estimation of the critical size for triply charged cluster ions. Utilizing a beam deflection method 19 it is possible to observe (for the first time) directly the asymmetric fission of multiply charged neon clusters right after the ionization event. The most abundant low mass fragment ion from this reaction process is the dimer ion. The yield of larger fragment ions decreases exponentially with the fragment size. The kinetic energy of the emitted low mass fragment ions is of the order of 200 meV which is surprisingly low when comparing the results with a simple point charge model taking into account the critical cluster sizes presently determined. (author)

  16. A singly charged ion source for radioactive 11C ion acceleration

    International Nuclear Information System (INIS)

    A new singly charged ion source using electron impact ionization has been developed to realize an isotope separation on-line system for simultaneous positron emission tomography imaging and heavy-ion cancer therapy using radioactive 11C ion beams. Low-energy electron beams are used in the electron impact ion source to produce singly charged ions. Ionization efficiency was calculated in order to decide the geometric parameters of the ion source and to determine the required electron emission current for obtaining high ionization efficiency. Based on these considerations, the singly charged ion source was designed and fabricated. In testing, the fabricated ion source was found to have favorable performance as a singly charged ion source

  17. A singly charged ion source for radioactive ¹¹C ion acceleration.

    Science.gov (United States)

    Katagiri, K; Noda, A; Nagatsu, K; Nakao, M; Hojo, S; Muramatsu, M; Suzuki, K; Wakui, T; Noda, K

    2016-02-01

    A new singly charged ion source using electron impact ionization has been developed to realize an isotope separation on-line system for simultaneous positron emission tomography imaging and heavy-ion cancer therapy using radioactive (11)C ion beams. Low-energy electron beams are used in the electron impact ion source to produce singly charged ions. Ionization efficiency was calculated in order to decide the geometric parameters of the ion source and to determine the required electron emission current for obtaining high ionization efficiency. Based on these considerations, the singly charged ion source was designed and fabricated. In testing, the fabricated ion source was found to have favorable performance as a singly charged ion source. PMID:26932062

  18. A singly charged ion source for radioactive 11C ion acceleration

    Science.gov (United States)

    Katagiri, K.; Noda, A.; Nagatsu, K.; Nakao, M.; Hojo, S.; Muramatsu, M.; Suzuki, K.; Wakui, T.; Noda, K.

    2016-02-01

    A new singly charged ion source using electron impact ionization has been developed to realize an isotope separation on-line system for simultaneous positron emission tomography imaging and heavy-ion cancer therapy using radioactive 11C ion beams. Low-energy electron beams are used in the electron impact ion source to produce singly charged ions. Ionization efficiency was calculated in order to decide the geometric parameters of the ion source and to determine the required electron emission current for obtaining high ionization efficiency. Based on these considerations, the singly charged ion source was designed and fabricated. In testing, the fabricated ion source was found to have favorable performance as a singly charged ion source.

  19. A singly charged ion source for radioactive {sup 11}C ion acceleration

    Energy Technology Data Exchange (ETDEWEB)

    Katagiri, K.; Noda, A.; Nagatsu, K.; Nakao, M.; Hojo, S.; Muramatsu, M.; Suzuki, K.; Wakui, T.; Noda, K. [National Institute of Radiological Sciences, 4-9-1 Anagawa, Inage-ku, Chiba-shi, Chiba 263-8555 (Japan)

    2016-02-15

    A new singly charged ion source using electron impact ionization has been developed to realize an isotope separation on-line system for simultaneous positron emission tomography imaging and heavy-ion cancer therapy using radioactive {sup 11}C ion beams. Low-energy electron beams are used in the electron impact ion source to produce singly charged ions. Ionization efficiency was calculated in order to decide the geometric parameters of the ion source and to determine the required electron emission current for obtaining high ionization efficiency. Based on these considerations, the singly charged ion source was designed and fabricated. In testing, the fabricated ion source was found to have favorable performance as a singly charged ion source.

  20. Electron emission and defect formation in the interaction of slow, highly charged ions with diamond surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Sideras-Haddad, E. [School of Physics, University of the Witwatersrand, Wits 2050, Johannesburg (South Africa)]. E-mail: haddade@physics.wits.ac.za; Schenkel, T. [E. O. Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Rebuli, D.B. [School of Physics, University of the Witwatersrand, Wits 2050, Johannesburg (South Africa); Persaud, A. [E. O. Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Shrivastava, S. [School of Physics, University of the Witwatersrand, Wits 2050, Johannesburg (South Africa); Schneider, D.H. [Lawrence Livermore National Laboratory, Livermore, CA 94550 (United States); Mwakikunga, B. [School of Physics, University of the Witwatersrand, Wits 2050, Johannesburg (South Africa)

    2007-03-15

    We report on electron emission and defect formation in the interaction between slow ({nu} {approx} 0.3 {nu}{sub Bohr}) highly charged ions (SHCI) with insulating (type IIa) and semiconducting (type IIb) diamonds. Electron emission induced by {sup 31}P {sup q+} (q = 5-13) and {sup 136}Xe {sup q+} (q = 34-44) with kinetic energies of 9 kV x q increase linearly with the ion charge states, reaching over 100 electrons per ion for high xenon charge states without surface passivation of the diamond with hydrogen. Yields from both diamond types are up to a factor of two higher than from reference metal surfaces. Crater like defects with diameters of 25-40 nm are formed by the impact of single Xe{sup 44+} ions. High secondary electron yields and single ion induced defects enable the formation of single dopant arrays on diamond surfaces.

  1. Ion-UHMA: a model for simulating the dynamics of neutral and charged aerosol particles.

    Energy Technology Data Exchange (ETDEWEB)

    Leppae, J.; Kerminen, V.-M. (Finnish Meteorological Institute, Climate Change Research, Helsinki (Finland)); Gagne, S.; Manninen, H. E.; Nieminen, T.; Kulmala, M. (Dept. of Physics, Univ. of Helsinki (Finland)); Laakso, L. (Dept. of Physics, Univ. of Helsinki (Finland); School of Physical and Chemical Sciences, North-West Univ. Potchefstroom (South Africa)); Korhonen, H. (Univ. of Kuopio, Dept. of Physics (Finland)); Lehtinen, K. E. J. (Univ. of Kuopio, Dept. of Physics (Finland); Finnish Meteorological Institute, Kuopio Unit (Finland))

    2009-07-01

    A new aerosol dynamical box model, Ion-UHMA (University of Helsinki Multicomponent Aerosol model for neutral and charged particles), is introduced in this paper. The model includes basic dynamical processes (condensation, coagulation and deposition) as well as ion-aerosol attachment and ion-ion recombination. The formation of particles is treated as model input or, alternatively, the model can be coupled with an existing nucleation model. Ion-UHMA was found to be able to reproduce qualitatively the measured time evolution of the particle number size distribution, when the particle formation and growth rates as well as concentrations of particles > 20 nm in diameter were taken from measurements. The simulated charging state of freshly formed particles during a new particle formation event evolved towards charge equilibrium in line with previously-derived analytical formulae. We provided a few illustrative examples to demonstrate possible applications, to which the Ion-UHMA model could be used in the near future. (orig.)

  2. Multiply-charged ion emission from a cyclotron-resonance-heated plasma ion source

    International Nuclear Information System (INIS)

    Electron cyclotron resonance heated ion sources have become the prominent electron-stripping device used to produce multiply-charged ions. These ions are required for many applications ranging from atomic physics research to cyclotron injection. Unfortunately, many of these sources are designed, built and operated based on empirical knowledge acquired from past or existing machines. Much research remains to be performed before a solid understanding of the physical processes governing these sources can be gained. The work presented here attempts to partially bridge the gap between application and understanding. A time-of-flight spectrometer diagnostic system was implemented on MIMI to measure the endloss current density for specific charge states flowing from the mirror. The method of acquiring many spectra in a given shot over a relatively short span of real time, and averaging them to produce one averaged spectrum has proven quite effective in reducing random signal fluctuations. Also, shot-to-shot reproducibility becomes possible with this method -- a difficult and most welcome result. Ion cyclotron heating has been shown to increase ion temperatures tens of eV. The resonant species typically experiences the greatest temperature increase but transfers much of its energy to the remainder of the distribution via collisions. These temperature increases are consistent with those expected from antenna loading computations. Modeling of the important physical processes occurring in the plasma yields results consistent with those measured with the time-of-flight spectrometer. 62 refs., 68 figs., 9 tabs

  3. Charge state breeding experiences and plans at TRIUMF

    Science.gov (United States)

    Ames, F.; Marchetto, M.; Mjøs, A.; Morton, A. C.

    2016-02-01

    At the Isotope Separation and ACceleration (ISAC) facility at TRIUMF, an electron cyclotron resonance ion source (ECRIS) has been set up for the charge state breeding of radioactive ions. In order to reduce background from stable ions generated in the ECRIS, several measures, including changing materials for the plasma chamber and the surrounding components, have been implemented. Further reduction has been achieved by using the post-accelerator chain as a mass filter. Since the implementation of those measures in 2013, physics experiments with accelerated radioactive isotopes of Rb, Sr, K, and Mg have been performed. In most cases, a charge breeding efficiency of several percent has been achieved. With the planned expansion of the isotope production capabilities at TRIUMF within the Advanced Rare IsotopE Laboratory project, two new target stations, one using photo-fission induced by a high-power electron beam at 50 MeV and the other one using 480 MeV protons as at ISAC, will be put into operation within the next 5 yr. Additionally, a new electron beam ion source (EBIS) based charge state breeding system will be installed. Background from such a source is expected to be much lower. The drawback is that for the efficient operation of such a system, pulsed beam operation is required, which makes the installation of an additional ion buncher in front of the EBIS necessary.

  4. Charge state breeding experiences and plans at TRIUMF

    International Nuclear Information System (INIS)

    At the Isotope Separation and ACceleration (ISAC) facility at TRIUMF, an electron cyclotron resonance ion source (ECRIS) has been set up for the charge state breeding of radioactive ions. In order to reduce background from stable ions generated in the ECRIS, several measures, including changing materials for the plasma chamber and the surrounding components, have been implemented. Further reduction has been achieved by using the post-accelerator chain as a mass filter. Since the implementation of those measures in 2013, physics experiments with accelerated radioactive isotopes of Rb, Sr, K, and Mg have been performed. In most cases, a charge breeding efficiency of several percent has been achieved. With the planned expansion of the isotope production capabilities at TRIUMF within the Advanced Rare IsotopE Laboratory project, two new target stations, one using photo-fission induced by a high-power electron beam at 50 MeV and the other one using 480 MeV protons as at ISAC, will be put into operation within the next 5 yr. Additionally, a new electron beam ion source (EBIS) based charge state breeding system will be installed. Background from such a source is expected to be much lower. The drawback is that for the efficient operation of such a system, pulsed beam operation is required, which makes the installation of an additional ion buncher in front of the EBIS necessary

  5. Charge state breeding experiences and plans at TRIUMF

    Energy Technology Data Exchange (ETDEWEB)

    Ames, F., E-mail: ames@triumf.ca; Marchetto, M.; Mjøs, A.; Morton, A. C. [TRIUMF, 4004 Wesbrook Mall, Vancouver, British Columbia V6T2A3 (Canada)

    2016-02-15

    At the Isotope Separation and ACceleration (ISAC) facility at TRIUMF, an electron cyclotron resonance ion source (ECRIS) has been set up for the charge state breeding of radioactive ions. In order to reduce background from stable ions generated in the ECRIS, several measures, including changing materials for the plasma chamber and the surrounding components, have been implemented. Further reduction has been achieved by using the post-accelerator chain as a mass filter. Since the implementation of those measures in 2013, physics experiments with accelerated radioactive isotopes of Rb, Sr, K, and Mg have been performed. In most cases, a charge breeding efficiency of several percent has been achieved. With the planned expansion of the isotope production capabilities at TRIUMF within the Advanced Rare IsotopE Laboratory project, two new target stations, one using photo-fission induced by a high-power electron beam at 50 MeV and the other one using 480 MeV protons as at ISAC, will be put into operation within the next 5 yr. Additionally, a new electron beam ion source (EBIS) based charge state breeding system will be installed. Background from such a source is expected to be much lower. The drawback is that for the efficient operation of such a system, pulsed beam operation is required, which makes the installation of an additional ion buncher in front of the EBIS necessary.

  6. Highly Charged Ions in Rare Earth Permanent Magnet Penning Traps

    OpenAIRE

    Guise, Nicholas D.; Brewer, Samuel M.; Tan, Joseph N.

    2012-01-01

    A newly constructed apparatus at the National Institute of Standards and Technology (NIST) is designed for the isolation, manipulation, and study of highly charged ions. Highly charged ions are produced in the NIST electron-beam ion trap (EBIT), extracted through a beamline that selects a single mass/charge species, then captured in a compact Penning trap. The magnetic field of the trap is generated by cylindrical NdFeB permanent magnets integrated into its electrodes. In a room-temperature p...

  7. Instantaneous charge state of Uranium projectiles in fully ionized plasmas from energy loss experiments

    CERN Document Server

    Morales, Roberto; Casas, David

    2016-01-01

    The instantaneous charge state of uranium ions traveling through a fully ionized hydrogen plasma has been theoretically studied and compared with one of the first energy loss experiments in plasmas, carried out at GSI-Darmstadt by Hoffmann \\textit{et al.} in the 90's. For this purpose, two different methods to estimate the instantaneous charge state of the projectile have been employed: (1) rate equations using ionization and recombination cross sections, and (2) equilibrium charge state formulas for plasmas. Also, the equilibrium charge state has been obtained using these ionization and recombination cross sections, and compared with the former equilibrium formulas. The equilibrium charge state of projectiles in plasmas is not always reached, it depends mainly on the projectile velocity and the plasma density. Therefore, a non-equilibrium or an instantaneous description of the projectile charge is necessary. The charge state of projectile ions cannot be measured, except after exiting the target, and experime...

  8. Neutralization Of Multiply Charged Rydberg Ions Interacting With Solid Surfaces Under The Grazing Incidence Geometry

    Science.gov (United States)

    Majkic, M. D.; Nedeljkovic, N. N.; Galijas, S. M. D.

    2010-07-01

    We elaborated the time-symmetric, two-state vector model to investigate the intermediate stages of the electron capture into the Rydberg states of multiply charged ions interacting with solid surface under the grazing incidence geometry. The neutralization distances for the ions XeZ+ interacting with Al-surface are calculated, for core charges Z ?[5,30]. The corresponding mean neutralization distances are in agreement with the data deduced from the measured kinetic energy gain due to the image acceleration of the ions.

  9. Possible diamond-like nanoscale structures induced by slow highly-charged ions on graphite (HOPG)

    International Nuclear Information System (INIS)

    The interaction between slow highly-charged ions (SHCI) of different charge states from an electron-beam ion trap and highly-oriented pyrolytic graphite (HOPG) surfaces is studied in terms of modification of electronic states at single-ion impact nanosize areas. Results are presented from AFM/STM analysis of the induced-surface topological features combined with Raman spectroscopy. I-V characteristics for a number of different impact regions were measured with STM and the results argue for possible formation of diamond-like nanoscale structures at the impact sites.

  10. Possible diamond-like nanoscale structures induced by slow highly-charged ions on graphite (HOPG)

    Energy Technology Data Exchange (ETDEWEB)

    Sideras-Haddad, E. [School of Physics, University of the Witwatersrand, Wits 2050, Johannesburg (South Africa); iThemba LABS for Accelerator Based Sciences, Johannesburg-Gauteng (South Africa)], E-mail: haddade@physics.wits.ac.za; Schenkel, T. [E.O. Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Shrivastava, S.; Makgato, T. [School of Physics, University of the Witwatersrand, Wits 2050, Johannesburg (South Africa); Batra, A.; Weis, C.D.; Persaud, A. [E.O. Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Erasmus, R.; Mwakikunga, B. [School of Physics, University of the Witwatersrand, Wits 2050, Johannesburg (South Africa)

    2009-08-15

    The interaction between slow highly-charged ions (SHCI) of different charge states from an electron-beam ion trap and highly-oriented pyrolytic graphite (HOPG) surfaces is studied in terms of modification of electronic states at single-ion impact nanosize areas. Results are presented from AFM/STM analysis of the induced-surface topological features combined with Raman spectroscopy. I-V characteristics for a number of different impact regions were measured with STM and the results argue for possible formation of diamond-like nanoscale structures at the impact sites.

  11. Possible Diamond-Like Nanoscale Structures Induced by Slow Highly-Charged Ions on Graphite (HOPG)

    Energy Technology Data Exchange (ETDEWEB)

    Sideras-Haddad, E.; Schenkel, T.; Shrivastava, S.; Makgato, T.; Batra, A.; Weis, C. D.; Persaud, A.; Erasmus, R.; Mwakikunga, B.

    2009-01-06

    The interaction between slow highly-charged ions (SHCI) of different charge states from an electron-beam ion trap and highly oriented pyrolytic graphite (HOPG) surfaces is studied in terms of modification of electronic states at single-ion impact nanosizeareas. Results are presented from AFM/STM analysis of the induced-surface topological features combined with Raman spectroscopy. I-V characteristics for a number of different impact regions were measured with STM and the results argue for possible formation of diamond-like nanoscale structures at the impact sites.

  12. Final report: Department of Energy grant to Kansas State University - J. R. Macdonald Laboratory. Atomic physics with highly charged ions: Supplementary request for Accelerator Improvement Project

    International Nuclear Information System (INIS)

    The following tasks for previous funding periods are sketched: LHe compressor relocation, LINAC RF electronics upgrade, tandem Van de Graaff foil changer; tandem Van de Graaff terminal pump installation; replace power transistors in magnet power supplies; new EBIS beam line vacuum system, EBIS beam optics upgrade, tandem Van de Graaff cryopumps, tandem upcharge system, PIG source for ion-ion system, LINAC beam line, EBIS beam optics and safety upgrade, EBIS beam power upgrade, ion-ion facility upgrade, ion-ion upgrade, new LINAC beamline, LINAC cryostat upgrade, LHe plant equipment, EBIS beamline upgrade. The task for this period, high voltage platform and ion-beam handling peripherals, is gone into in greater detail

  13. Online Identification with Reliability Criterion and State of Charge Estimation Based on a Fuzzy Adaptive Extended Kalman Filter for Lithium-Ion Batteries

    Directory of Open Access Journals (Sweden)

    Zhongwei Deng

    2016-06-01

    Full Text Available In the field of state of charge (SOC estimation, the Kalman filter has been widely used for many years, although its performance strongly depends on the accuracy of the battery model as well as the noise covariance. The Kalman gain determines the confidence coefficient of the battery model by adjusting the weight of open circuit voltage (OCV correction, and has a strong correlation with the measurement noise covariance (R. In this paper, the online identification method is applied to acquire the real model parameters under different operation conditions. A criterion based on the OCV error is proposed to evaluate the reliability of online parameters. Besides, the equivalent circuit model produces an intrinsic model error which is dependent on the load current, and the property that a high battery current or a large current change induces a large model error can be observed. Based on the above prior knowledge, a fuzzy model is established to compensate the model error through updating R. Combining the positive strategy (i.e., online identification and negative strategy (i.e., fuzzy model, a more reliable and robust SOC estimation algorithm is proposed. The experiment results verify the proposed reliability criterion and SOC estimation method under various conditions for LiFePO4 batteries.

  14. New Supercharging Reagents Produce Highly Charged Protein Ions in Native Mass Spectrometry

    OpenAIRE

    Going, Catherine C; Xia, Zijie; Williams, Evan R.

    2015-01-01

    The effectiveness of two new supercharging reagents for producing highly charged ions by electrospray ionization (ESI) from aqueous solutions in which proteins have native structures and reactivities were investigated. In aqueous solution, 2-thiophenone and 4-hydroxymethyl-1,3-dioxolan-2-one (HD) at a concentration of 2% by volume can increase the average charge of cytochrome c and myoglobin by up to 163%, resulting in even higher charge states than those that are produced from water/methanol...

  15. Space-charge limits of ion sensitive probes

    Science.gov (United States)

    Brunner, D.; LaBombard, B.; Ochoukov, R.; Sullivan, R.; Whyte, D.

    2013-12-01

    Ion sensitive probes (ISPs) are used to measure ion temperature and plasma potential in magnetized plasmas. Their operation relies on the difference in electron and ion Larmor radii to preferentially collect the ion species on a recessed electrode. Because of their simple two-electrode construction and optimal geometry for heat flux handling they are an attractive probe to use in the high heat flux boundary of magnetic confinement fusion experiments. However, the integrity of its measurements is rarely, if ever, checked under such conditions. Recent measurements with an ISP in the Alcator C-Mod tokamak have shown that its ion current is space-charge limited and thus its current-voltage (I-V) response does not contain information on the ion temperature. We numerically solve a 1D Vlasov-Poisson model of ion collection to determine how much bias is needed to overcome space-charge effects and regain the classic I-V characteristic with an exponential decay. Prompted by the observations of space charge in C-Mod, we have performed a survey of ISP measurements reported in the literature. Evidence of space-charge limited current collection is found on many probes, with few authors noting its presence. Some probes are able to apparently exceed the classic 1D space-charge limit because electrons can E × B drift into the probe volume, partially reducing the net ion charge; it is argued that this does not, however, change the basic problem that space charge compromises the measurement of ion temperature. Guidance is given for design of ISPs to minimize the effects of space charge.

  16. New state of nuclear matter: Nearly perfect fluid of quarks and gluons in heavy-ion collisions at RHIC energies. From charged particle density to jet quenching

    Science.gov (United States)

    Nouicer, R.

    2016-03-01

    This article reviews several important results from RHIC experiments and discusses their implications. They were obtained in a unique environment for studying QCD matter at temperatures and densities that exceed the limits wherein hadrons can exist as individual entities and raises to prominence the quark-gluon degrees of freedom. These findings are supported by major experimental observations via measuring of the bulk properties of particle production, particle ratios and chemical freeze-out conditions, and elliptic flow; followed by hard probe measurements: high- pT hadron suppression, dijet fragment azimuthal correlations, and heavy-flavor probes. These measurements are presented for particles of different species as a function of system sizes, collision centrality, and energy carried out in RHIC experiments. The results reveal that a dense, strongly interacting medium is created in central Au+Au collisions at sqrt{s_{NN}} = 200 GeV at RHIC. This revelation of a new state of nuclear matter has also been observed in measurements at the LHC. Further, the IP-Glasma model coupled with viscous hydrodynamic models, which assumes the formation of a QGP, reproduces well the experimental flow results from Au+Au at sqrt{s_{NN}} = 200 GeV. This implies that the fluctuations in the initial geometry state are important and the created medium behaves as a nearly perfect liquid of nuclear matter because it has an extraordinarily low ratio of shear viscosity to entropy density, η/s≈ 0.12. However, these discoveries are far from being fully understood. Furthermore, recent experimental results from RHIC and LHC in small p+A, d+ Au and 3He+Au collision systems provide brand new insight into the role of initial and final state effects. These have proven to be interesting and more surprising than originally anticipated; and could conceivably shed new light in our understanding of collective behavior in heavy-ion physics. Accordingly, the focus of the experiments at both

  17. Element- and charge-state-resolved ion energies in the cathodic arc plasma from composite AlCr cathodes in argon, nitrogen and oxygen atmospheres

    OpenAIRE

    Franz, Robert; Polcik, Peter; Anders, André

    2014-01-01

    The energy distribution functions of ions in the cathodic arc plasma using composite AlCr cathodes were measured as a function of the background gas pressure in the range 0.5 to 3.5 Pa for different cathode compositions and gas atmospheres. The most abundant aluminium ions were Al$^{+}$ regardless of the background gas species, whereas Cr$^{2+}$ ions were dominating in Ar and N$_2$ and Cr$^{+}$ in O$_2$ atmospheres. The energy distributions of the aluminium and chromium ions typically consist...

  18. Excitation of atoms and molecules in collisions with fast, highly charged ions

    International Nuclear Information System (INIS)

    This paper discusses the following topics: charge distributions for Ar recoil-ions produced in one- and two-electron capture collisions by Oq+ projectiles; charge distributions of He, Ne, and Ar recoil-ions produced in collisions with 10 to 30 MeV/u N7+ ions; studies of recoil ions produced in collisions of 40 MeV Ar13+ with atomic and molecular targets; two-fragment coincidence studies of molecular dissociation induced by heavy ion collisions; resonant electron transfer to double K-vacancy states in oxygen compounds; quenching of metastable states in fast Mg projectiles; and design and construction of an atomic physics beamline for the ECR ion source

  19. Charge exchange between singly ionized helium ions

    International Nuclear Information System (INIS)

    The plane-wave Born approximation was used to evaluate the charge transfer cross sections for the reaction He+ + He+ → He++ + He. The charge transfer cross section is graphed as a function of incident energy and compared with experimental measurements

  20. A low-charge-state injector linac for ATLAS

    International Nuclear Information System (INIS)

    The design of a low-charge-state linac which is capable of accelerating, for example, 132Sn1+ for injection into the existing heavy-ion linac ATLAS is discussed. The injector linac is intended for radioactive beam applications, and will accelerate a low- charge-state beam to energies of 500 keV/nucleon, at which point the ions can be stripped to charge states sufficiently high to be injected into ATLAS. A primary design goal has been to extend the very good longitudinal beam quality typical of ATLAS to low charge state beams. The proposed injector linac consists of several elements. First is a gridded-gap four-harmonic buncher and a short (normally-conducting) 12 MHz RFQ structure, both operating on a 350 kV open-air variable-voltage platform. Then comes an array of 24 Mhz and 48 Mhz superconducting interdigital accelerating structures interspersed with superconducting quadrupole transverse focusing elements. Numerical ray-tracing studies indicate that a transverse acceptance greater than 0.25π mm-mrad can be obtained while simultaneously limiting longitudinal emittance growth to a very few keV-nsec

  1. Investigations on Cooling Mechanisms of Highly Charged Ions at HITRAP

    Science.gov (United States)

    Maero, Giancarlo; Herfurth, Frank; Kester, Oliver; Kluge, H.-Jürgen; Koszudowski, Stephen; Quint, Wolfgang; Schwarz, Stefan

    2009-03-01

    The upcoming facility HITRAP (Highly Charged Ion TRAP) at GSI will enable high-precision atomic-physics investigations on heavy, highly charged ions at extremely low energies. Species up to U92+ will be produced at the GSI accelerator complex by stripping of relativistic ions and injected into the Experimental Storage Ring (ESR) where they are electron-cooled and decelerated to 4 MeV/u. After ejection out of the ESR and further deceleration in a linear decelerator bunches of 105 ions will be injected into a Penning trap and cooled to 4 K via electron and resistive cooling. Simulations with a Particle-In-Cell (PIC) code have been carried out to study the dynamics of the ion cloud in the Cooler Trap with focus on resistive cooling in presence of space charge.

  2. Collision phenomena involving highly-charged ions in astronomical objects

    Science.gov (United States)

    Chutjian, A.

    2001-01-01

    A description of the role of highly charged ions in various astronomical objects; includes the use of critical quantities such as cross sections for excitation, charge-exchange, X-ray emission, radiative recombination (RR) and dielectronic recombination (DR); and lifetimes, branching ratios, and A-values.

  3. Autoionization of helium following excitation by fast, multiply charged ions

    International Nuclear Information System (INIS)

    Using two parallel plate electrostatic spectrometers, the authors have measured the autoionization spectra of doubly-excited helium, following excitation by charged, 700 to 3500 KeV lithium ions produced by the Dynamitron. In particular, they studied the effect of projectile nuclear charge on the helium autoionization profiles and the continuum in which they are embedded

  4. Excitation and ionization of highly charged ions by electron impact

    International Nuclear Information System (INIS)

    Two approaches for very rapid calculation of atomic data for high temperature plasma modeling have been developed. The first uses hydrogenic basis states and has been developed and applied in many papers discussed in previous progress reports. Hence, it is only briefly discussed here. The second is a very rapid, yet accurate, fully relativistic approach that has been developed over the past two or three years. It is described in more detail. Recently it has been applied to large scale production of atomic data. Specifically, it has been used to calculate relativistic distorted wave collision strengths and oscillator strengths for the following: all transitions from the ground level to the n=3 and 4 excited levels in the 71 Neon-like ions with nuclear charge number Z in the range 22 ≤ Z ≤ 92; all transitions among the 2s1/2, 2p1/2 and 2p3/2 levels and from them to all nlj levels with n=3,4 and 5 in the 85 Li-like ions with 8 ≤ Z ≤ 92; all transitions among the 3s1/2, 3p3/2, 3d3/2 and 3d5/2 levels and from them to all nlj levels with n=4 and 5 in the 71 Na-like ions with 22 ≤ Z ≤ 92; and all transitions among 4s1/2, 4p1/2, 4p3/2, 4d3/2, 4d5/2, 4f5/2 and 4f7/2 levels and from them to all nlj levels with n=5 in the 33 Cu-like ions with 60 ≤ Z ≤ 92. Also the program has been extended to give cross-sections for excitation to specific magnetic sublevels of the target ion by an electron beam and very recently it has been extended to give relativistic distorted wave cross sections for ionization of highly charged ions by electron impact

  5. Correlated charge-changing ion-atom collisions

    International Nuclear Information System (INIS)

    This report summarizes the progress and accomplishments in accelerator atomic physics research supported by DOE grant DE-FG02-87ER13778 from February 16, 1990 through February 15, 1993. This work involves the experimental investigation of atomic interactions in collisions of charged projectiles with neutral targets or electrons, with particular emphasis on two-electron interactions and electron-correlation effects. The processes studied are of interest both from fundamental and applied points of view. In the latter case, results are obtained which are relevant to the understanding of laboratory and astrophysical plasmas, highly-excited (Rydberg) and continuum states of atoms and ions, atomic structure effects, the interaction of ions with surfaces, and the development of heavy-ion storage-rings. The results obtained have provided the basis for several M.A. thesis projects at Western Michigan and several Ph.D. dissertation projects are currently underway. Summaries of work completed and work in progress are given below in Section II. This research has resulted in 26 papers (in print and in press), 12 invited presentations at national and international meetings, and 28 contributed presentations as detailed in Section III

  6. Cryogenic linear Paul trap for cold highly charged ion experiments

    DEFF Research Database (Denmark)

    Schwarz, Maria; Versolato, Oscar; Windberger, Alexander;

    2012-01-01

    Storage and cooling of highly charged ions require ultra-high vacuum levels obtainable by means of cryogenic methods. We have developed a linear Paul trap operating at 4 K capable of very long ion storage times of about 30 h. A conservative upper bound of the H2 partial pressure of about 10−15 mbar...

  7. A compact source for bunches of singly charged atomic ions

    Science.gov (United States)

    Murböck, T.; Schmidt, S.; Andelkovic, Z.; Birkl, G.; Nörtershäuser, W.; Vogel, M.

    2016-04-01

    We have built, operated, and characterized a compact ion source for low-energy bunches of singly charged atomic ions in a vacuum beam line. It is based on atomic evaporation from an electrically heated oven and ionization by electron impact from a heated filament inside a grid-based ionization volume. An adjacent electrode arrangement is used for ion extraction and focusing by applying positive high-voltage pulses to the grid. The method is particularly suited for experimental environments which require low electromagnetic noise. It has proven simple yet reliable and has been used to produce μs-bunches of up to 106 Mg+ ions at a repetition rate of 1 Hz. We present the concept, setup and characterizing measurements. The instrument has been operated in the framework of the SpecTrap experiment at the HITRAP facility at GSI/FAIR to provide Mg+ ions for sympathetic cooling of highly charged ions by laser-cooled 24Mg+.

  8. Intense beam production of highly charged heavy ions by the superconducting electron cyclotron resonance ion source SECRAL.

    Science.gov (United States)

    Zhao, H W; Sun, L T; Zhang, X Z; Guo, X H; Cao, Y; Lu, W; Zhang, Z M; Yuan, P; Song, M T; Zhao, H Y; Jin, T; Shang, Y; Zhan, W L; Wei, B W; Xie, D Z

    2008-02-01

    There has been increasing demand to provide higher beam intensity and high enough beam energy for heavy ion accelerator and some other applications, which has driven electron cyclotron resonance (ECR) ion source to produce higher charge state ions with higher beam intensity. One of development trends for highly charged ECR ion source is to build new generation ECR sources by utilization of superconducting magnet technology. SECRAL (superconducting ECR ion source with advanced design in Lanzhou) was successfully built to produce intense beams of highly charged ion for Heavy Ion Research Facility in Lanzhou (HIRFL). The ion source has been optimized to be operated at 28 GHz for its maximum performance. The superconducting magnet confinement configuration of the ion source consists of three axial solenoid coils and six sextupole coils with a cold iron structure as field booster and clamping. An innovative design of SECRAL is that the three axial solenoid coils are located inside of the sextupole bore in order to reduce the interaction forces between the sextupole coils and the solenoid coils. For 28 GHz operation, the magnet assembly can produce peak mirror fields on axis of 3.6 T at injection, 2.2 T at extraction, and a radial sextupole field of 2.0 T at plasma chamber wall. During the commissioning phase at 18 GHz with a stainless steel chamber, tests with various gases and some metals have been conducted with microwave power less than 3.5 kW by two 18 GHz rf generators. It demonstrates the performance is very promising. Some record ion beam intensities have been produced, for instance, 810 e microA of O(7+), 505 e microA of Xe(20+), 306 e microA of Xe(27+), and so on. The effect of the magnetic field configuration on the ion source performance has been studied experimentally. SECRAL has been put into operation to provide highly charged ion beams for HIRFL facility since May 2007. PMID:18315105

  9. Reducing Space Charge Effects in a Linear Ion Trap by Rhombic Ion Excitation and Ejection

    Science.gov (United States)

    Zhang, Xiaohua; Wang, Yuzhuo; Hu, Lili; Guo, Dan; Fang, Xiang; Zhou, Mingfei; Xu, Wei

    2016-07-01

    Space charge effects play important roles in ion trap operations, which typically limit the ion trapping capacity, dynamic range, mass accuracy, and resolving power of a quadrupole ion trap. In this study, a rhombic ion excitation and ejection method was proposed to minimize space charge effects in a linear ion trap. Instead of applying a single dipolar AC excitation signal, two dipolar AC excitation signals with the same frequency and amplitude but 90° phase difference were applied in the x- and y-directions of the linear ion trap, respectively. As a result, mass selective excited ions would circle around the ion cloud located at the center of the ion trap, rather than go through the ion cloud. In this work, excited ions were then axially ejected and detected, but this rhombic ion excitation method could also be applied to linear ion traps with ion radial ejection capabilities. Experiments show that space charge induced mass resolution degradation and mass shift could be alleviated with this method. For the experimental conditions in this work, space charge induced mass shift could be decreased by ~50%, and the mass resolving power could be improved by ~2 times at the same time.

  10. Comparision of multiply charged ion productions by different lasers

    Czech Academy of Sciences Publication Activity Database

    Láska, Leoš; Krása, Josef; Rohlena, Karel; Parys, P.; Wolowski, J.; Woryna, E.

    Bologna : Italian Physical Society, 2001 - (Gammino, S.; Ciavola, G.), s. 39-44 - (Conference Proceedings.. 72). [Workshop on the Production of Intense Beams of Highly Charged Ions . Catania (IT), 24.09.2000-27.09.2000] R&D Projects: GA MŠk LN00A100 Grant ostatní: HPRI(XE) CT-1999-00053 Institutional research plan: CEZ:AV0Z1010921 Keywords : iodine laser * laser produce ions * ion characteristics Subject RIV: BJ - Thermodynamics

  11. Fast electronic resistance switching involving hidden charge density wave states

    Science.gov (United States)

    Vaskivskyi, I.; Mihailovic, I. A.; Brazovskii, S.; Gospodaric, J.; Mertelj, T.; Svetin, D.; Sutar, P.; Mihailovic, D.

    2016-05-01

    The functionality of computer memory elements is currently based on multi-stability, driven either by locally manipulating the density of electrons in transistors or by switching magnetic or ferroelectric order. Another possibility is switching between metallic and insulating phases by the motion of ions, but their speed is limited by slow nucleation and inhomogeneous percolative growth. Here we demonstrate fast resistance switching in a charge density wave system caused by pulsed current injection. As a charge pulse travels through the material, it converts a commensurately ordered polaronic Mott insulating state in 1T-TaS2 to a metastable electronic state with textured domain walls, accompanied with a conversion of polarons to band states, and concurrent rapid switching from an insulator to a metal. The large resistance change, high switching speed (30 ps) and ultralow energy per bit opens the way to new concepts in non-volatile memory devices manipulating all-electronic states.

  12. Fast electronic resistance switching involving hidden charge density wave states.

    Science.gov (United States)

    Vaskivskyi, I; Mihailovic, I A; Brazovskii, S; Gospodaric, J; Mertelj, T; Svetin, D; Sutar, P; Mihailovic, D

    2016-01-01

    The functionality of computer memory elements is currently based on multi-stability, driven either by locally manipulating the density of electrons in transistors or by switching magnetic or ferroelectric order. Another possibility is switching between metallic and insulating phases by the motion of ions, but their speed is limited by slow nucleation and inhomogeneous percolative growth. Here we demonstrate fast resistance switching in a charge density wave system caused by pulsed current injection. As a charge pulse travels through the material, it converts a commensurately ordered polaronic Mott insulating state in 1T-TaS2 to a metastable electronic state with textured domain walls, accompanied with a conversion of polarons to band states, and concurrent rapid switching from an insulator to a metal. The large resistance change, high switching speed (30 ps) and ultralow energy per bit opens the way to new concepts in non-volatile memory devices manipulating all-electronic states. PMID:27181483

  13. Positron-impact ionization of highly charged ions in lowest-order QED theory

    International Nuclear Information System (INIS)

    Lowest-order QED theory using distorted-wave states is applied to the calculation of positron-impact ionization cross sections for highly charged atomic ions. Electron and positron ionization cross sections for atomic ions are predicted to differ by substantial amounts in the threshold region. For highly charged ions like U90+, the smaller positron ionization cross section is more strongly affected by transverse photon interactions than the corresponding electron ionization cross section. At twice the threshold for U90+ ionization, the annihilation terms are found to reduce the positron cross section by about 12%

  14. Charge equilibrium of a laser-generated carbon-ion beam in warm dense matter

    International Nuclear Information System (INIS)

    Using ion carbon beams generated by high intensity short pulse lasers we perform measurements of single shot mean charge equilibration in cold or isochorically heated solid density aluminum matter. We demonstrate that plasma effects in such matter heated up to 1 eV do not significantly impact the equilibration of carbon ions with energies 0.045-0.5 MeV/nucleon. Furthermore, these measurements allow for a first evaluation of semiempirical formulas or ab initio models that are being used to predict the mean of the equilibrium charge state distribution for light ions passing through warm dense matter. (authors)

  15. Investigation of charge balance in ion accelerator TEMP-4M

    Science.gov (United States)

    Khailov, I. P.; Pak, V. G.

    2014-10-01

    The paper presents the results of a study on the balance of charge in accelerator TEMP-4M operating in double-pulse mode with resistance load and ion diode. Crucially, it was found, that during the switching there is no losses of accumulated charge. It means, that all accumulated charge transferred to the load. However when the charge is transferred from the Marx generator to Blumlein line the half of accumulated charge is lost. Calibration of diagnostic equipment showed a good agreement between the calculated and experimental values of voltage and current. It means, that our diagnostic system is correct for registration parameters of the ion accelerator. A distinctive feature of the ion accelerators with self-magnetically insulated diode is that there is no need to use additional energy source for the creation of an external magnetic field. That's why the efficiency of ion diodes with an external magnetic field is not more than 10-15%. The efficiency of energy conversion in self-magnetically insulated diodes will be determined by not only the efficiency of the diode, but the energy losses in the units of the accelerator. The aim of the researches is the analysis of the balance of charge in units of the ion beams pulsed generator and definition of the most significant channels of energy loss.

  16. Coherent pion production in heavy ion charge exchange reactions

    International Nuclear Information System (INIS)

    We report the first observation of coherent pion production induced by a heavy ion charge exchange reaction. The (12C,12N) reaction [D. Bachelier et al., Phys. Lett. B 172 (1986) 23; M. Roy-Stephan et al., Nucl. Phys. A 488 (1988) 178] at 1.1 GeV/nucleon has been used to shine negative (off-shell) pions on nuclei and observe (on-shell) pions, leaving the target nucleus in its ground state. The experiment was performed at the Laboratoire National Saturne with the SPES4-π setup [Laurent Farhi PHD thesis IPNO-T97-12, Universite d'Orsay, 1997; Rasmus Dahl Ph.D., Niels Bohr Institutet, Copenhagen (1999)

  17. The ReA electron-beam ion trap charge breeder for reacceleration of rare isotopes

    Science.gov (United States)

    Lapierre, A.; Schwarz, S.; Kittimanapun, K.; Fogleman, J.; Krause, S.; Nash, S.; Rencsok, R.; Tobos, L.; Perdikakis, G.; Portillo, M.; Rodriguez, J. A.; Wittmer, W.; Wu, X.; Bollen, G.; Leitner, D.; Syphers, M.; ReA Team

    2013-04-01

    ReA is a post-accelerator at the National Superconducting Cyclotron Laboratory at Michigan State University. ReA is designed to reaccelerate rare isotopes to energies of a few MeV/u following production by projectile fragmentation and thermalization in a gas cell. The facility consists of four main components: an electron-beam ion trap (EBIT) charge breeder, an achromatic charge-over-mass (Q/A) separator, a radio-frequency quadrupole accelerator, and a superconducting radio-frequency linear accelerator. The EBIT charge breeder was specifically designed to efficiently capture continuous beams of singly charged ions injected at low energy (breed in less than 50 ms, and extract highly charged ions to the Q/A separator for charge-state selection and reacceleration through the accelerator structures. The use of highly charged ions to reach high beam energies is a key aspect that makes ReA a compact and cost-efficient post-accelerator. The EBIT is characterized by a high-current electron gun, a long multi-electrode trap structure and a dual magnet to provide both the high electron-beam current density necessary for fast charge breeding of short-lived isotopes as well as the high capture probability of injected beams. This paper presents an overview and the status of the ReA EBIT, which has extracted for reacceleration tests stable 20Ne8+ ion beams produced from injected gas and more recently 39K16+ beams by injecting stable 39,41K+ ions from an external ion source.

  18. Projectile charge state dependent sputtering of solid surfaces

    CERN Document Server

    Hayderer, G

    2000-01-01

    dependence on the ion kinetic energy. This new type of potential sputtering not only requires electronic excitation of the target material, but also the formation of a collision cascade within the target in order to initiate the sputtering process and has therefore been termed kinetically assisted potential sputtering. In order to study defects induced by potential sputtering on the atomic scale we performed measurements of multiply charged Ar ion irradiated HOPG (highly oriented pyrolitic graphite) samples with scanning tunneling microscopy (STM). The only surface defects found in the STM images are protrusions. The mean diameter of the defects increases with projectile charge state while the height of the protrusions stays roughly the same indicating a possible pre-equilibrium effect of the stopping of slow multiply charged projectiles in HOPG. Total sputter yields for impact of slow singly and multiply charged ions on metal- (Au), oxide- (Al2O3, MgO) and alkali-halide surfaces (LiF) have been measured as a...

  19. Magnetohydrodynamics and charged currents in heavy ion collisions

    International Nuclear Information System (INIS)

    The hot QCD matter produced in any heavy ion collision with a nonzero impact parameter is produced within a strong magnetic field. We study the imprint the magnetic fields produced in non-central heavy ion collisions leave on the azimuthal distributions and correlations of the produced charged hadrons. The magnetic field is time-dependent and the medium is expanding, which leads to the induction of charged currents due to the combination of Faraday and Hall effects. We find that these currents result in a charge-dependent directed flow v1 that is odd in rapidity and odd under charge exchange. It can be detected by measuring correlations between the directed flow of charged hadrons at different rapidities, 〈v1±(y1)v1±(y2)〉

  20. Fast and efficient charge breeding of the Californium rare isotope breeder upgrade electron beam ion source

    Energy Technology Data Exchange (ETDEWEB)

    Ostroumov, P. N., E-mail: ostroumov@anl.gov; Barcikowski, A.; Dickerson, C. A.; Perry, A.; Sharamentov, S. I.; Vondrasek, R. C.; Zinkann, G. P. [Argonne National Laboratory, Argonne, Illinois 60439 (United States); Pikin, A. I. [Brookhaven National Laboratory, Upton, New York 11973 (United States)

    2015-08-15

    The Electron Beam Ion Source (EBIS), developed to breed Californium Rare Isotope Breeder Upgrade (CARIBU) radioactive beams at Argonne Tandem Linac Accelerator System (ATLAS), is being tested off-line. A unique property of the EBIS is a combination of short breeding times, high repetition rates, and a large acceptance. Overall, we have implemented many innovative features during the design and construction of the CARIBU EBIS as compared to the existing EBIS breeders. The off-line charge breeding tests are being performed using a surface ionization source that produces singly charged cesium ions. The main goal of the off-line commissioning is to demonstrate stable operation of the EBIS at a 10 Hz repetition rate and a breeding efficiency into single charge state higher than 15%. These goals have been successfully achieved and exceeded. We have measured (20% ± 0.7%) breeding efficiency into the single charge state of 28+ cesium ions with the breeding time of 28 ms. In general, the current CARIBU EBIS operational parameters can provide charge breeding of any ions in the full mass range of periodic table with high efficiency, short breeding times, and sufficiently low charge-to-mass ratio, 1/6.3 for the heaviest masses, for further acceleration in ATLAS. In this paper, we discuss the parameters of the EBIS and the charge breeding results in a pulsed injection mode with repetition rates up to 10 Hz.

  1. Fast and efficient charge breeding of the Californium rare isotope breeder upgrade electron beam ion source

    International Nuclear Information System (INIS)

    The Electron Beam Ion Source (EBIS), developed to breed Californium Rare Isotope Breeder Upgrade (CARIBU) radioactive beams at Argonne Tandem Linac Accelerator System (ATLAS), is being tested off-line. A unique property of the EBIS is a combination of short breeding times, high repetition rates, and a large acceptance. Overall, we have implemented many innovative features during the design and construction of the CARIBU EBIS as compared to the existing EBIS breeders. The off-line charge breeding tests are being performed using a surface ionization source that produces singly charged cesium ions. The main goal of the off-line commissioning is to demonstrate stable operation of the EBIS at a 10 Hz repetition rate and a breeding efficiency into single charge state higher than 15%. These goals have been successfully achieved and exceeded. We have measured (20% ± 0.7%) breeding efficiency into the single charge state of 28+ cesium ions with the breeding time of 28 ms. In general, the current CARIBU EBIS operational parameters can provide charge breeding of any ions in the full mass range of periodic table with high efficiency, short breeding times, and sufficiently low charge-to-mass ratio, 1/6.3 for the heaviest masses, for further acceleration in ATLAS. In this paper, we discuss the parameters of the EBIS and the charge breeding results in a pulsed injection mode with repetition rates up to 10 Hz

  2. Fast and efficient charge breeding of the Californium rare isotope breeder upgrade electron beam ion source.

    Science.gov (United States)

    Ostroumov, P N; Barcikowski, A; Dickerson, C A; Perry, A; Pikin, A I; Sharamentov, S I; Vondrasek, R C; Zinkann, G P

    2015-08-01

    The Electron Beam Ion Source (EBIS), developed to breed Californium Rare Isotope Breeder Upgrade (CARIBU) radioactive beams at Argonne Tandem Linac Accelerator System (ATLAS), is being tested off-line. A unique property of the EBIS is a combination of short breeding times, high repetition rates, and a large acceptance. Overall, we have implemented many innovative features during the design and construction of the CARIBU EBIS as compared to the existing EBIS breeders. The off-line charge breeding tests are being performed using a surface ionization source that produces singly charged cesium ions. The main goal of the off-line commissioning is to demonstrate stable operation of the EBIS at a 10 Hz repetition rate and a breeding efficiency into single charge state higher than 15%. These goals have been successfully achieved and exceeded. We have measured (20% ± 0.7%) breeding efficiency into the single charge state of 28+ cesium ions with the breeding time of 28 ms. In general, the current CARIBU EBIS operational parameters can provide charge breeding of any ions in the full mass range of periodic table with high efficiency, short breeding times, and sufficiently low charge-to-mass ratio, 1/6.3 for the heaviest masses, for further acceleration in ATLAS. In this paper, we discuss the parameters of the EBIS and the charge breeding results in a pulsed injection mode with repetition rates up to 10 Hz. PMID:26329185

  3. Adsorption of Potassium and Calcium Ions by Variable Charge Soils

    Institute of Scientific and Technical Information of China (English)

    LIHONG-YAN; JIGUO-LIANG

    1992-01-01

    Interactions of potassium and calcium ions with four typical variable charge soils in South China were examined by measuring pK-0.5pCa value with a potassium ion-selective electrode and a calcium ion-selective electrode,and pK value with a potassium ion-selective electrode.The results showed that adsorption of potassium and calcium ions increased with soil suspension pH,and the tendency of the pK-0.5pCa value changing with pH differed with respect to pH range and potassium to calcium ratio.Adsorption of equal amount of calcium and potassium ions led to release of an identical number of protons,suggesting similar adsorption characteristics of these two ions when adsorbed by variable charge soils.Compared with red soil,latosol and lateritic red soil had higher adsorption selectivities for calcium ion.The red soil had a greater affinity for potassium ion than that for calcium ion at low concentration,which seems to result from its possession of 2:1 type minerals,such as vermiculite and mica with a high affinity for potassium ion.The results indicated that adsorption of potassium and calcium ions by the variable charge soils was chiefly caused by the electrostatic attraction between the cations and the soil surfaces.Moreover,it was found that sulfate could affect the adsorption by changing soil surface properties and by forming ion-pair.

  4. Adsorption of Potassium and Sodium Ions by Variable Charge Soils

    Institute of Scientific and Technical Information of China (English)

    LIHONG-YAN; JIGUO-LIANG

    1992-01-01

    Adsorption of potassium and sodium ions by four typical variable charge soils of South China was studied.The results indicated that the variable charge soils saturated with H and Al showed a much higher preference for potassium ions relative to sodium ions,and this tendence could not be changed by such factors as the pH,the concentration of the cations,the dielectric constant of solvent,the accompanying anions and the iron oxide content etc.,suggesting that this difference in affinity is caused by the difference in the nature of the two cations.It was observed that a negative adsorption of sodium ions by latosol and lateritic red soil in a mixed system containing equal amount of potassium and sodium ions at low pH,which is caused by a competitive adsorption of potassium and sodium ions and repulsion of positive charge on the surfaces of soil particles for cations.The adsorption of potassium and sodium ions increased with the decreases in the dielectric constant of solvent and the iron oxide content.Sulfate affected the adsorption of potassium and sodium ions through changing the surface properties of the soils.

  5. Electron capture by highly charged low-velocity ions

    International Nuclear Information System (INIS)

    This paper describes the use of a fast heavy ion beam to produce, by bombardment of gaseous targets, highly-charged low-velocity recoil ions, and the use of these secondary ions in turn as projectiles in studies of electron capture and ionization in low-energy collision systems. The interest in collisions involving low-energy highly-charged projectiles comes both from the somewhat simplifying aspects of the physics which attend the long-range capture and from applications to fusion plasmas, astrophysics and more speculative technology such as the production of X-ray lasers. The ions of interest in such applications should have both electronic excitation and center-of-mass energies in the keV range and cannot be produced by simply stripping fast heavy ion beams. Several novel types of ion source have been developed to produce low-energy highly-charged ions, of which the secondary ion recoil source discussed in this paper is one. (Auth.)

  6. Study on space charge compensation in negative hydrogen ion beam

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, A. L.; Chen, J. E. [University of Chinese Academy of Sciences, Beijing 100049 (China); State Key Laboratory of Nuclear Physics and Technology, Institute of Heavy Ion Physics, School of Physics, Peking University, Beijing 100871 (China); Peng, S. X., E-mail: sxpeng@pku.edu.cn; Ren, H. T.; Zhang, T.; Zhang, J. F.; Xu, Y.; Guo, Z. Y. [State Key Laboratory of Nuclear Physics and Technology, Institute of Heavy Ion Physics, School of Physics, Peking University, Beijing 100871 (China)

    2016-02-15

    Negative hydrogen ion beam can be compensated by the trapping of ions into the beam potential. When the beam propagates through a neutral gas, these ions arise due to gas ionization by the beam ions. However, the high neutral gas pressure may cause serious negative hydrogen ion beam loss, while low neutral gas pressure may lead to ion-ion instability and decompensation. To better understand the space charge compensation processes within a negative hydrogen beam, experimental study and numerical simulation were carried out at Peking University (PKU). The simulation code for negative hydrogen ion beam is improved from a 2D particle-in-cell-Monte Carlo collision code which has been successfully applied to H{sup +} beam compensated with Ar gas. Impacts among ions, electrons, and neutral gases in negative hydrogen beam compensation processes are carefully treated. The results of the beam simulations were compared with current and emittance measurements of an H{sup −} beam from a 2.45 GHz microwave driven H{sup −} ion source in PKU. Compensation gas was injected directly into the beam transport region to modify the space charge compensation degree. The experimental results were in good agreement with the simulation results.

  7. Study on space charge compensation in negative hydrogen ion beam

    Science.gov (United States)

    Zhang, A. L.; Peng, S. X.; Ren, H. T.; Zhang, T.; Zhang, J. F.; Xu, Y.; Guo, Z. Y.; Chen, J. E.

    2016-02-01

    Negative hydrogen ion beam can be compensated by the trapping of ions into the beam potential. When the beam propagates through a neutral gas, these ions arise due to gas ionization by the beam ions. However, the high neutral gas pressure may cause serious negative hydrogen ion beam loss, while low neutral gas pressure may lead to ion-ion instability and decompensation. To better understand the space charge compensation processes within a negative hydrogen beam, experimental study and numerical simulation were carried out at Peking University (PKU). The simulation code for negative hydrogen ion beam is improved from a 2D particle-in-cell-Monte Carlo collision code which has been successfully applied to H+ beam compensated with Ar gas. Impacts among ions, electrons, and neutral gases in negative hydrogen beam compensation processes are carefully treated. The results of the beam simulations were compared with current and emittance measurements of an H- beam from a 2.45 GHz microwave driven H- ion source in PKU. Compensation gas was injected directly into the beam transport region to modify the space charge compensation degree. The experimental results were in good agreement with the simulation results.

  8. Study on space charge compensation in negative hydrogen ion beam

    International Nuclear Information System (INIS)

    Negative hydrogen ion beam can be compensated by the trapping of ions into the beam potential. When the beam propagates through a neutral gas, these ions arise due to gas ionization by the beam ions. However, the high neutral gas pressure may cause serious negative hydrogen ion beam loss, while low neutral gas pressure may lead to ion-ion instability and decompensation. To better understand the space charge compensation processes within a negative hydrogen beam, experimental study and numerical simulation were carried out at Peking University (PKU). The simulation code for negative hydrogen ion beam is improved from a 2D particle-in-cell-Monte Carlo collision code which has been successfully applied to H+ beam compensated with Ar gas. Impacts among ions, electrons, and neutral gases in negative hydrogen beam compensation processes are carefully treated. The results of the beam simulations were compared with current and emittance measurements of an H− beam from a 2.45 GHz microwave driven H− ion source in PKU. Compensation gas was injected directly into the beam transport region to modify the space charge compensation degree. The experimental results were in good agreement with the simulation results

  9. Projectile charge state dependence of M-shell ionization of Au, Pb, Bi, and U by 1.42-MeV/amu fluorine ions

    International Nuclear Information System (INIS)

    The present study was undertaken to determine the direct ionization and electron capture contributions to vacancy production in the M-shells of 79Au, 82Pb, 83Bi and 92U for incident 199F ions. M-shell x-ray production cross sections have been measured for 1.42-MeV/amu 199Fq+ ions for q = 4,5,6,8,9. Enhancements in the target x-ray production cross sections were observed for projectiles with one and two K-shell vacancies over those without K-shell vacancies. Direct ionization and electron capture contributions to the vacancy production were extracted from the data and compared to the plane wave Born approximation and to the Oppenheimer-Brinkman-Kramers calculations of Nikolaev, respectively

  10. Fragmentation of phosphorylated and singly charged peptide ions via interaction with metastable atoms.

    Science.gov (United States)

    Berkout, Vadym D; Doroshenko, Vladimir M

    2008-12-01

    Fragmentation of phosphorylated peptide ions via interaction with electronically excited metastable argon atoms was studied in a linear trap - time-of-flight mass spectrometer. Doubly charged ions of phosphorylated peptides from an Enolase digest were produced by electrospray ionization and subjected to a metastable atom beam in the linear trap. The metastable argon atoms were generated using a glow-discharge source. An intensive series of c- and z- ions were observed in all cases, with the phosphorylation group intact. The formation of molecular radical cations with reduced charge indicated that an electron transfer from a highly excited metastable state of argon to the peptide cation occurred. Additionally, singly charged Bradykinin, Substance P and Fibrinopeptide A molecular ions were fragmented via interaction with electronically excited metastable helium atoms. The fragmentation mechanism was different in this case and involved Penning ionization. PMID:19956340

  11. Aberrations due to solenoid focusing of a multiply charged high-current ion beam

    CERN Document Server

    Grégoire, G; Lisi, N; Schnuriger, J C; Scrivens, R; Tambini, J

    2000-01-01

    At the output of a laser ion source, a high current of highly charged ions with a large range of charge states is available. The focusing of such a beam by magnetic elements causes a nonlinear space-charge field to develop which can induce large aberrations and emittance growth in the beam. Simulation of the beam from the CERN laser ion source will be presented for an ideal magnetic and electrostatic system using a radially symmetric model. In addition, the three dimensional software KOBRA3 is used for the simulation of the solenoid line. The results of these simulations will be compared with experiments performed on the CERN laser ion source with solenoids (resulting in a hollow beam) and a series of gridded electrostatic lenses. (5 refs).

  12. Atomic physics with highly charged ions

    International Nuclear Information System (INIS)

    This report discusses: One electron outer shell processes in fast ion-atom collisions; role of electron-electron interaction in two-electron processes; multi-electron processes at low energy; multi-electron processes at high energy; inner shell processes; molecular fragmentation studies; theory; and, JRM laboratory operations

  13. Spectroscopy of highly charged multi-electron ions

    International Nuclear Information System (INIS)

    Systematic studies of highs charged neonlike and nickellike ions as well as several open-shell ions performed on an electron beam ion trap are described and used to assess the accuracy of structure calculations of multi-electron ions. Discrepancies are found that can be attributed to inaccuracies in accounting for electron correlations and in estimating quantum electrodynamical effects. Documenting the effects of level crossings, we demonstrate that these discrepancies are compounded by uncertainties in assigning the respective contributions from quantum electrodynamics to each of the two strongly interacting levels undergoing the crossing

  14. Medium effects on charged pion ratio in heavy ion collisions

    CERN Document Server

    Ko, Che Ming; Xu, Jun

    2010-01-01

    We have recently studied in the delta-resonance--nucleon-hole model the dependence of the pion spectral function in hot dense asymmetric nuclear matter on the charge of the pion due to the pion p-wave interaction in nuclear medium. In a thermal model, this isospin-dependent effect enhances the ratio of negatively charged to positively charged pions in neutron-rich nuclear matter, and the effect is comparable to that due to the uncertainties in the theoretically predicted stiffness of nuclear symmetry energy at high densities. This effect is, however, reversed if we also take into account the s-wave interaction of the pion in nuclear medium as given by chiral perturbation theory, resulting instead in a slightly reduced ratio of negatively charged to positively charged pions. Relevance of our results to the determination of the nuclear symmetry energy from the ratio of negatively to positively charged pions produced in heavy ion collisions is discussed.

  15. Medium effects on charged pion ratio in heavy ion collisions

    International Nuclear Information System (INIS)

    We have recently studied in the delta-resonance–nucleon-hole model the dependence of the pion spectral function in hot dense asymmetric nuclear matter on the charge of the pion due to the pion p-wave interaction in nuclear medium. In a thermal model, this isospin-dependent effect enhances the ratio of negatively charged to positively charged pions in neutron-rich nuclear matter, and the effect is comparable to that due to the uncertainties in the theoretically predicted stiffness of nuclear symmetry energy at high densities. This effect is, however, reversed if we also take into account the s-wave interaction of the pion in nuclear medium as given by chiral perturbation theory, resulting instead in a slightly reduced ratio of negatively charged to positively charged pions. Relevance of our results to the determination of the nuclear symmetry energy from the ratio of negatively to positively charged pions produced in heavy ion collisions is discussed. (author)

  16. Emission of ions and charged soot particles by aircraft engines

    Directory of Open Access Journals (Sweden)

    A. Sorokin

    2003-01-01

    Full Text Available In this article, a model which examines the formation and evolution of chemiions in an aircraft engine is proposed. This model which includes chemiionisation, electron thermo-emission, electron attachment to soot particles and to neutral molecules, electron-ion and ion-ion recombination, ion-soot interaction, allows the determination of the ion concentration at the exit of the combustor and at the nozzle exit of the engine. It also allows the determination of the charge of the soot particles. For the engine considered, the upper limit for the ion emission index EIi is of the order of (2-5 x1016 ions/kg-fuel if ion-soot interactions are ignored and the introduction of ion-soot interactions lead about to a 50% reduction. The results also show that most of the soot particles are either positively or negatively charged, the remaining neutral particles representing approximately 20% of the total particles. A comparison of the model results with the available ground-based experimental data obtained on the ATTAS research aircraft engines during the SULFUR experiments (Schumann, 2002 shows an excellent agreement.

  17. Electrokinetic inversion of ion screening charges in nano-channels

    CERN Document Server

    Zhu, Xin; Ni, Sheng; Zhang, Xingye; Liu, Yang

    2016-01-01

    This work studies a counter-intuitive but basic process of ionic screening in nano-fluidic channels. Numerical simulations and perturbation analysis reveal that, under significant electrokinetic transport, the ion screening charges can be locally inverted in the channels: their charge sign becomes the same as that of the channel surface charges. The process is identified to originate from the coupling of longitudinal transport and junction electrostatics. This finding may revise the common understanding of ionic screening in nano-channels and indicates that their ion selectivity can be locally changed by transport. Furthermore, the charge inversion process results in a body force torque on channel fluids, which is a possible mechanism for vortex generation in the channels.

  18. Studies of emittance of multiply charged ions extracted from high temperature superconducting electron cyclotron resonance ion source, PKDELIS

    International Nuclear Information System (INIS)

    For the high current injector project at Inter University Accelerator Centre, a high temperature superconducting electron cyclotron resonance (ECR) ion source, PKDELIS, would provide the high charge state ions. The emittance of the ECR ion source is an important parameter to design further beam transport system and to match the acceptances of the downstream radio frequency quadrupole and drift tube linac accelerators of the high current injector. The emittance of the analyzed beam of PKDELIS ECR source has been measured utilizing the three beam size technique. A slit and two beam profile monitors positioned at fixed distances from each other were used to measure the beam size. The digitized beam profiles have been analyzed to determine the emittance of various multiply charged ions. The variation of emittance with gas mixing, ultrahigh frequency power, and extraction energy are discussed in this presentation.

  19. QED corrections to atomic wavefunctions in highly charged ions

    International Nuclear Information System (INIS)

    Bound electron states in highly charged ions are strongly influenced by the effects of relativity and quantum electrodynamics (QED). These effects induce shifts of the binding energies as well as corrections to observables related to atomic processes. In this work a numerical procedure is described and implemented in which the QED effects are treated as corrections to relativistic bound-state wavefunctions. This approach, which is based on the recently developed covariant evolution-operator formalism, allows for a merging of QED with the standard methods of many-body perturbation theory. In particular, it enables an evaluation of the combined effect of QED and electron correlation in few-electron systems. Numerical results for this effect are presented for the ground state energy of helium-like ions. A detailed analysis of the contribution from the electron self-energy is carried out in both the Feynman and Coulomb gauge. It is found that the Feynman gauge suffers from large numerical cancellations and acquires significant contributions from terms involving multiple interactions with the nuclear potential (the so-called many-potential terms), while the Coulomb gauge is well suited for an approximate treatment based on terms involving only freely propagating electrons (the zero-potential terms). With the help of QED-corrected wavefunctions it is also possible to compute corrections to observables in basic atomic processes. In this work some of the one-loop QED corrections (those derivable from perturbed wavefunctions and energies) to the differential cross section and distribution of polarization in radiative recombination of initially bare uranium nuclei are evaluated, as well as the corresponding corrections to the ratio τE1/τM2 of the electric dipole and magnetic quadrupole transition amplitudes in the 2p3/2→1s radiative decay of hydrogenlike uranium. The results from these calculations are all of the expected magnitude, namely on the order of the fine

  20. QED corrections to atomic wavefunctions in highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Holmberg, Johan

    2015-11-18

    Bound electron states in highly charged ions are strongly influenced by the effects of relativity and quantum electrodynamics (QED). These effects induce shifts of the binding energies as well as corrections to observables related to atomic processes. In this work a numerical procedure is described and implemented in which the QED effects are treated as corrections to relativistic bound-state wavefunctions. This approach, which is based on the recently developed covariant evolution-operator formalism, allows for a merging of QED with the standard methods of many-body perturbation theory. In particular, it enables an evaluation of the combined effect of QED and electron correlation in few-electron systems. Numerical results for this effect are presented for the ground state energy of helium-like ions. A detailed analysis of the contribution from the electron self-energy is carried out in both the Feynman and Coulomb gauge. It is found that the Feynman gauge suffers from large numerical cancellations and acquires significant contributions from terms involving multiple interactions with the nuclear potential (the so-called many-potential terms), while the Coulomb gauge is well suited for an approximate treatment based on terms involving only freely propagating electrons (the zero-potential terms). With the help of QED-corrected wavefunctions it is also possible to compute corrections to observables in basic atomic processes. In this work some of the one-loop QED corrections (those derivable from perturbed wavefunctions and energies) to the differential cross section and distribution of polarization in radiative recombination of initially bare uranium nuclei are evaluated, as well as the corresponding corrections to the ratio τ{sub E1}/τ{sub M2} of the electric dipole and magnetic quadrupole transition amplitudes in the 2p{sub 3/2}→1s radiative decay of hydrogenlike uranium. The results from these calculations are all of the expected magnitude, namely on the order

  1. Spectator charge splitting of directed flow in heavy ion collisions

    CERN Document Server

    Szczurek, Antoni

    2013-01-01

    We estimate the effect of the spectator charge on distortion of single charged pion distributions as well as on azimuthal anisotropies in heavy ion collisions. A large electromagnetic effect on directed flow $v_1$ is predicted in good agreement with existing WA98 as well as RHIC data. This effect results in a splitting of $v_1$ for positive and negative pions. Detailed analysis of this phenomenon may provide new information on the collision dynamics.

  2. Production of highly charged ion beams with SECRAL.

    Science.gov (United States)

    Sun, L T; Zhao, H W; Lu, W; Zhang, X Z; Feng, Y C; Li, J Y; Cao, Y; Guo, X H; Ma, H Y; Zhao, H Y; Shang, Y; Ma, B H; Wang, H; Li, X X; Jin, T; Xie, D Z

    2010-02-01

    Superconducting electron cyclotron resonance ion source with advanced design in Lanzhou (SECRAL) is an all-superconducting-magnet electron cyclotron resonance ion source (ECRIS) for the production of intense highly charged ion beams to meet the requirements of the Heavy Ion Research Facility in Lanzhou (HIRFL). To further enhance the performance of SECRAL, an aluminum chamber has been installed inside a 1.5 mm thick Ta liner used for the reduction of x-ray irradiation at the high voltage insulator. With double-frequency (18+14.5 GHz) heating and at maximum total microwave power of 2.0 kW, SECRAL has successfully produced quite a few very highly charged Xe ion beams, such as 10 e microA of Xe(37+), 1 e microA of Xe(43+), and 0.16 e microA of Ne-like Xe(44+). To further explore the capability of the SECRAL in the production of highly charged heavy metal ion beams, a first test run on bismuth has been carried out recently. The main goal is to produce an intense Bi(31+) beam for HIRFL accelerator and to have a feel how well the SECRAL can do in the production of very highly charged Bi beams. During the test, though at microwave power less than 3 kW, more than 150 e microA of Bi(31+), 22 e microA of Bi(41+), and 1.5 e microA of Bi(50+) have been produced. All of these results have again demonstrated the great capability of the SECRAL source. This article will present the detailed results and brief discussions to the production of highly charged ion beams with SECRAL. PMID:20192339

  3. Production of highly charged ion beams with SECRAL

    International Nuclear Information System (INIS)

    Superconducting electron cyclotron resonance ion source with advanced design in Lanzhou (SECRAL) is an all-superconducting-magnet electron cyclotron resonance ion source (ECRIS) for the production of intense highly charged ion beams to meet the requirements of the Heavy Ion Research Facility in Lanzhou (HIRFL). To further enhance the performance of SECRAL, an aluminum chamber has been installed inside a 1.5 mm thick Ta liner used for the reduction of x-ray irradiation at the high voltage insulator. With double-frequency (18+14.5 GHz) heating and at maximum total microwave power of 2.0 kW, SECRAL has successfully produced quite a few very highly charged Xe ion beams, such as 10 e μA of Xe37+, 1 e μA of Xe43+, and 0.16 e μA of Ne-like Xe44+. To further explore the capability of the SECRAL in the production of highly charged heavy metal ion beams, a first test run on bismuth has been carried out recently. The main goal is to produce an intense Bi31+ beam for HIRFL accelerator and to have a feel how well the SECRAL can do in the production of very highly charged Bi beams. During the test, though at microwave power less than 3 kW, more than 150 e μA of Bi31+, 22 e μA of Bi41+, and 1.5 e μA of Bi50+ have been produced. All of these results have again demonstrated the great capability of the SECRAL source. This article will present the detailed results and brief discussions to the production of highly charged ion beams with SECRAL.

  4. Charge separation with fluctuating domains in relativistic heavy-ion collisions

    OpenAIRE

    Shou, Qi-Ye; Ma, Guo-Liang; Ma, Yu-Gang

    2014-01-01

    Charge separation induced by the chiral magnetic effect suggested that some ${\\cal P}$- or ${\\cal CP}$-odd metastable domains could be produced in a QCD vacuum in the early stage of relativistic heavy-ion collisions. Based on a multi-phase transport model, our results suggest that a domain-based scenario with final state interactions can describe the solenoidal tracker at RHIC detector (STAR) measurements of both same- and opposite-charge azimuthal angle correlations, $$, in Au+Au collisions ...

  5. Design of a 4D Emittance Measurement Device for High Charge State ECR Ion Sources%高电荷态ECR离子源引出束流4D发射度测量仪设计

    Institute of Scientific and Technical Information of China (English)

    赵阳阳; 赵红卫; 孙良亭; 杨尧; 王云; 曹云

    2013-01-01

    For the purpose of on-line beam quality diagnostics and transverse emittance coupling investigation of the ion beams delivered by an Electron Cyclotron Resonance (ECR) ion source, a real-time 4D Pepper Pot type emittance scanner is under development at IMP(Institute of Moden Physics, Chinese Academy of Sciences). The high charge state ECR ion source at IMP could produce CW or pulsed heavy ion beam intensities in the range of 1 eµA∼1 emA with the kinetic energy of 10∼35 keV/q, which needs the design of the Pepper Pot scanner to be optimized accordingly. The Pepper Pot scanner has many features, such as very short response time and wide dynamic working range that the device could be applied. Since intense heavy ion beam bombardment is expected for this device, the structure and the material selection for the device is specially considered during the design, and a feasible solution to analyze the pictures acquired after the data acquisition is also made.%为了进一步探究高电荷态电子回旋共振(ECR)离子源引出束流品质和横向相空间耦合情况,根据中国科学院近代物理研究所高电荷态离子源引出束流发射度测量需求,针对束流流强为1 eµA∼1 emA,能量范围为10∼35 keV/q的直流或脉冲高电荷态重离子束,设计了一台实时四维Pepper-pot发射度测量仪。该Pepper-pot型发射度测量仪具有响应时间快和工作范围宽等特点。针对强流重离子束诊断的特点,在结构与材料选择上做了设计与优化,并对获得图像的处理方法提出了具体的解决办法。

  6. Ionization Efficiency of Doubly Charged Ions Formed from Polyprotic Acids in Electrospray Negative Mode.

    Science.gov (United States)

    Liigand, Piia; Kaupmees, Karl; Kruve, Anneli

    2016-07-01

    The ability of polyprotic acids to give doubly charged ions in negative mode electrospray was studied and related to physicochemical properties of the acids via linear discriminant analysis (LDA). It was discovered that the compound has to be strongly acidic (low pK a1 and pK a2) and to have high hydrophobicity (logP ow) to become multiply charged. Ability to give multiply charged ions in ESI/MS cannot be directly predicted from the solution phase acidities. Therefore, for the first time, a quantitative model to predict the charge state of the analyte in ESI/MS is proposed and validated for small anions. Also, a model to predict ionization efficiencies of these analytes was developed. Results indicate that acidity of the analyte, its octanol-water partition coefficient, and charge delocalization are important factors that influence ionization efficiencies as well as charge states of the analytes. The pH of the solvent was also found to be an important factor influencing the ionization efficiency of doubly charged ions. Graphical Abstract ᅟ. PMID:27044024

  7. Ionization Efficiency of Doubly Charged Ions Formed from Polyprotic Acids in Electrospray Negative Mode

    Science.gov (United States)

    Liigand, Piia; Kaupmees, Karl; Kruve, Anneli

    2016-04-01

    The ability of polyprotic acids to give doubly charged ions in negative mode electrospray was studied and related to physicochemical properties of the acids via linear discriminant analysis (LDA). It was discovered that the compound has to be strongly acidic (low pK a1 and pK a2) and to have high hydrophobicity (logP ow) to become multiply charged. Ability to give multiply charged ions in ESI/MS cannot be directly predicted from the solution phase acidities. Therefore, for the first time, a quantitative model to predict the charge state of the analyte in ESI/MS is proposed and validated for small anions. Also, a model to predict ionization efficiencies of these analytes was developed. Results indicate that acidity of the analyte, its octanol-water partition coefficient, and charge delocalization are important factors that influence ionization efficiencies as well as charge states of the analytes. The pH of the solvent was also found to be an important factor influencing the ionization efficiency of doubly charged ions.

  8. Properties of Laser-Produced Highly Charged Heavy Ions for Direct Injection Scheme

    CERN Document Server

    Sakakibara, Kazuhiko; Hayashizaki, Noriyosu; Ito, Taku; Kashiwagi, Hirotsugu; Okamura, Masahiro

    2005-01-01

    To accelerate highly charged intense ion beam, we have developed the Direct Plasma Injection Scheme (DPIS) with laser ion source. In this scheme an ion beam from a laser ion source is injected directly to a RFQ linac without a low energy beam transport (LEBT) and the beam loss in the LEBT can be avoided. We achieved high current acceleration of carbon ions (60mA) by DPIS with the high current optimized RFQ. As the next setp we will use heavier elements like Ag, Pb, Al and Cu as target in LIS (using CO2, Nd-YAG or other laser) for DPIS and will examine properties of laser-produced plasma (the relationship of between charge state and laser power density, the current dependence of the distance from the target, etc).

  9. Intercombination lines in highly charged Al- and Si-like ions

    International Nuclear Information System (INIS)

    Delayed spectroscopy techniques have been used to study the isoelectronic development for Al-like and Si-like intercombination line wavelengths. The ions studied range from Kr to Nb. The trend established for the quantity (Eobs -Ecalc)/ζ, (E being the transition energy and ζ the effective charge), shows that the available calculated data are not useful in identifying such intercombination lines for high Z ions. In the case of the Si-like intercombination lines the difference in wavelength between experiment and calculation is around 4 A for Nb27+ and this difference increases for higher Z ions. The line identifications were aided by recording spectra for different charge state distributions of the ions after the exciter foil. The experiments were done using ion beams from the RILAC accelerator at RIKEN. (orig.)

  10. Interaction of low-energy highly charged ions with matter

    International Nuclear Information System (INIS)

    The thesis presented herein deals with experimental studies of the interaction between highly charged ions and neutral matter at low collision energies. The energy range investigated is of great interest for the understanding of both charge exchange reactions between ions comprising the solar wind and various astrophysical gases, as well as the creation of near-surface nanostructures. Over the course of this thesis an experimental setup was constructed, capable of reducing the kinetic energy of incoming ions by two orders of magnitude and finally focussing the decelerated ion beam onto a solid or gaseous target. A coincidence method was employed for the simultaneous detection of photons emitted during the charge exchange process together with the corresponding projectile ions. In this manner, it was possible to separate reaction channels, whose superposition presumably propagated large uncertainties and systematic errors in previous measurements. This work has unveiled unexpectedly strong contributions of slow radiative decay channels and clear evidence of previously only postulated decay processes in charge exchange-induced X-ray spectra. (orig.)

  11. Polarization and charge transfer in the hydration of chloride ions

    International Nuclear Information System (INIS)

    A theoretical study of the structural and electronic properties of the chloride ion and water molecules in the first hydration shell is presented. The calculations are performed on an ensemble of configurations obtained from molecular dynamics simulations of a single chloride ion in bulk water. The simulations utilize the polarizable AMOEBA force field for trajectory generation and MP2-level calculations are performed to examine the electronic structure properties of the ions and surrounding waters in the external field of more distant waters. The ChelpG method is employed to explore the effective charges and dipoles on the chloride ions and first-shell waters. The quantum theory of atoms in molecules (QTAIM) is further utilized to examine charge transfer from the anion to surrounding water molecules. The clusters extracted from the AMOEBA simulations exhibit high probabilities of anisotropic solvation for chloride ions in bulk water. From the QTAIM analysis, 0.2 elementary charges are transferred from the ion to the first-shell water molecules. The default AMOEBA model overestimates the average dipole moment magnitude of the ion compared to the quantum mechanical value. The average magnitude of the dipole moment of the water molecules in the first shell treated at the MP2-level, with the more distant waters handled with an AMOEBA effective charge model, is 2.67 D. This value is close to the AMOEBA result for first-shell waters (2.72 D) and is slightly reduced from the bulk AMOEBA value (2.78 D). The magnitude of the dipole moment of the water molecules in the first solvation shell is most strongly affected by the local water-water interactions and hydrogen bonds with the second solvation shell, rather than by interactions with the ion.

  12. Polarization and charge transfer in the hydration of chloride ions

    Science.gov (United States)

    Zhao, Zhen; Rogers, David M.; Beck, Thomas L.

    2010-01-01

    A theoretical study of the structural and electronic properties of the chloride ion and water molecules in the first hydration shell is presented. The calculations are performed on an ensemble of configurations obtained from molecular dynamics simulations of a single chloride ion in bulk water. The simulations utilize the polarizable AMOEBA force field for trajectory generation and MP2-level calculations are performed to examine the electronic structure properties of the ions and surrounding waters in the external field of more distant waters. The ChelpG method is employed to explore the effective charges and dipoles on the chloride ions and first-shell waters. The quantum theory of atoms in molecules (QTAIM) is further utilized to examine charge transfer from the anion to surrounding water molecules. The clusters extracted from the AMOEBA simulations exhibit high probabilities of anisotropic solvation for chloride ions in bulk water. From the QTAIM analysis, 0.2 elementary charges are transferred from the ion to the first-shell water molecules. The default AMOEBA model overestimates the average dipole moment magnitude of the ion compared to the quantum mechanical value. The average magnitude of the dipole moment of the water molecules in the first shell treated at the MP2-level, with the more distant waters handled with an AMOEBA effective charge model, is 2.67 D. This value is close to the AMOEBA result for first-shell waters (2.72 D) and is slightly reduced from the bulk AMOEBA value (2.78 D). The magnitude of the dipole moment of the water molecules in the first solvation shell is most strongly affected by the local water-water interactions and hydrogen bonds with the second solvation shell, rather than by interactions with the ion.

  13. Space-charge effects in Penning ion traps

    Czech Academy of Sciences Publication Activity Database

    Porobic, T.; Beck, M.; Breitenfeldt, M.; Couratin, C.; Finlay, P.; Knecht, A.; Fabian, X.; Friedag, P.; Flechard, X.; Lienard, E.; Ban, G.; Zákoucký, Dalibor; Soti, G.; Van Gorp, S.; Weinheimer, C.; Wursten, E.; Severijns, N.

    2015-01-01

    Roč. 785, JUN (2015), s. 153-162. ISSN 0168-9002 R&D Projects: GA MŠk LA08015; GA MŠk(CZ) LG13031 Institutional support: RVO:61389005 Keywords : Penning trap * space-charge * magnetron motion * ion trapping * buffer gas cooling * ion cyclotron resonance Subject RIV: BG - Nuclear, Atomic and Molecular Physics, Colliders Impact factor: 1.216, year: 2014

  14. Convoy electron emission following ionization of highly-charged ions excited by resonant coherent excitation

    Science.gov (United States)

    Suda, S.; Nakano, Y.; Metoki, K.; Shindo, T.; Ohtsuki, S.; Azuma, T.; Hatakeyama, A.; Komaki, K.; Nakai, Y.; Takada, E.; Murakami, T.

    2012-11-01

    Projectile ionization of highly-charged Ar and Fe ions in the excited states passing relativistically fast through a thin crystalline foil was experimentally studied. We selectively controlled the population of the excited states of the projectiles, and their alignment by choosing a specific m-state through three-dimensional resonant coherent excitation technique by periodical electric fields in a crystalline. We measured energy-differential spectra of electron emission released from projectiles at zero degree. Under the resonance condition, we found an evident enhancement of the convoy electron yield, which reflects the electron momentum distribution of the initial bound state of the excited ions.

  15. Spatial distribution of charged particles along the ion-optical axis in electron cyclotron resonance ion sources. Experimental results

    International Nuclear Information System (INIS)

    The experimental determination of the spatial distribution of charged particles along the ion-optical axis in electron cyclotron resonance ion sources (ECRIS) defines the focus of this thesis. The spatial distributions of different ion species were obtained in the object plane of the bending magnet (∼45 cm downstream from the plasma electrode) and in the plane of the plasma electrode itself, both in high spatial resolution. The results show that each of the different ion species forms a bloated, triangular structure in the aperture of the plasma electrode. The geometry and the orientation of these structures are defined by the superposition of the radial and axial magnetic fields. The radial extent of each structure is defined by the charge of the ion. Higher charge states occupy smaller, more concentrated structures. The total current density increases towards the center of the plasma electrode. The circular and star-like structures that can be observed in the beam profiles of strongly focused, extracted ion beams are each dominated by ions of a single charge state. In addition, the spatially resolved current density distribution of charged particles in the plasma chamber that impinge on the plasma electrode was determined, differentiating between ions and electrons. The experimental results of this work show that the electrons of the plasma are strongly connected to the magnetic field lines in the source and thus spatially well confined in a triangular-like structure. The intensity of the electrons increases towards the center of the plasma electrode and the plasma chamber, as well. These electrons are surrounded by a spatially far less confined and less intense ion population. All the findings mentioned above were already predicted in parts by simulations of different groups. However, the results presented within this thesis represent the first (and by now only) direct experimental verification of those predictions and are qualitatively transferable to other

  16. Spatial distribution of charged particles along the ion-optical axis in electron cyclotron resonance ion sources. Experimental results

    Energy Technology Data Exchange (ETDEWEB)

    Panitzsch, Lauri

    2013-02-08

    The experimental determination of the spatial distribution of charged particles along the ion-optical axis in electron cyclotron resonance ion sources (ECRIS) defines the focus of this thesis. The spatial distributions of different ion species were obtained in the object plane of the bending magnet ({approx}45 cm downstream from the plasma electrode) and in the plane of the plasma electrode itself, both in high spatial resolution. The results show that each of the different ion species forms a bloated, triangular structure in the aperture of the plasma electrode. The geometry and the orientation of these structures are defined by the superposition of the radial and axial magnetic fields. The radial extent of each structure is defined by the charge of the ion. Higher charge states occupy smaller, more concentrated structures. The total current density increases towards the center of the plasma electrode. The circular and star-like structures that can be observed in the beam profiles of strongly focused, extracted ion beams are each dominated by ions of a single charge state. In addition, the spatially resolved current density distribution of charged particles in the plasma chamber that impinge on the plasma electrode was determined, differentiating between ions and electrons. The experimental results of this work show that the electrons of the plasma are strongly connected to the magnetic field lines in the source and thus spatially well confined in a triangular-like structure. The intensity of the electrons increases towards the center of the plasma electrode and the plasma chamber, as well. These electrons are surrounded by a spatially far less confined and less intense ion population. All the findings mentioned above were already predicted in parts by simulations of different groups. However, the results presented within this thesis represent the first (and by now only) direct experimental verification of those predictions and are qualitatively transferable to

  17. Mass and charge distribution in heavy-ion collisions

    International Nuclear Information System (INIS)

    A statistical model based on the independent particle picture is used to calculate mass and charge distributions in deep inelastic heavy-ion collisions. Different assumptions on volume and charge equilibrations are compared with measured variances of charge distributions. One combination of assumptions is clearly favoured by experiment, and gives a reasonable description of the variance versus energy loss curves up to energy losses of about 200 MeV in the heavy systems Kr+Ho and Xe+Bi, and up to about 60 MeV for the light system Ar+Ca

  18. High-resolution mobility analysis of charge-reduced electrosprayed protein ions.

    Science.gov (United States)

    Fernandez de la Mora, Juan

    2015-04-01

    Many mobility studies (IMS) of electrospray ions with charge states z reduced to unity have shown a singular ability to analyze large protein complexes and viruses, though with wide mobility peaks (fwhm ∼ 20%). Here we confirm that this limitation arises primarily when early charge reduction precedes drop evaporation (suppressing secondary atomization by the usual sequence of many Coulomb explosions). By drying before neutralizing, we achieve a protein fwhm of ∼3.7%. A positively biased electrospraying capillary is coaxial with a cylindrical charge-reduction (CR) chamber coated with radioactive Ni-63 (10 mCi) that fills the CR chamber with a bipolar ionic atmosphere. A screen interposed between the spraying capillary and the CR chamber limits penetration of the neutralizing anions into the electrospray (ES) chamber, precluding destabilization of the ES tip, even when brought very close to the grid to enhance ion transmission. As ES cations cross the grid, driven by their own space charge, they recombine with CR ions reducing their charge state as well as space charge dispersion. The setup is tested with the protein ovalbumin (MW ∼ 44.3 kDa) and its clusters up to the tetramer, by analyzing the charge-reduced ions with a differential mobility analyzer (DMA). At gas sample flow rates of ∼1 L/min, the dominant peaks are singly charged (z = 1). They are widened by clustering of involatile solution impurities, depending on spray quality and solution cleanness, with fwhm as small as 3.7% achieved in desalted and acidified solutions. When using sharp nanospray capillaries, the grid may be removed, resulting in ∼2-fold increased ion transmission. In the absence of the grid, however, spray stability and quality are often compromised, even with capillary tip diameters as small as 30 μm. PMID:25803189

  19. Selection of charge methods for lithium ion batteries by considering diffusion induced stress and charge time

    Science.gov (United States)

    Lu, Bo; Song, Yicheng; Zhang, Junqian

    2016-07-01

    This article demonstrates the design of charging strategies for lithium ion batteries with considering the balance between diffusion induced stress and total charge time for two- and three-stage charge methods. For the two-stage galvanostatic-potentiostatic charge method the low mechanical stress can be achieved without increasing total charge time by switching the galvanostatic to the potentiostatic at the time moment when the lithium concentration at the surface of particles reaches the limit cbarsurf = 0 . A three-stage method, which consists of an initial galvanostatic stage of high current, a galvanostatic stage of low current and a potentiostatic ending stage, is suggested. Employing the initial galvanostatic stage of high current is helpful not only in accelerating the charge process, but also in controlling the mechanical stress once the electrical current and time duration of the initial galvanostatic stage are properly designed.

  20. High-precision metrology of highly charged ions via relativistic resonance fluorescence

    OpenAIRE

    Postavaru, O; Harman, Z.; Keitel, C. H.

    2010-01-01

    Resonance fluorescence of laser-driven highly charged ions is studied in the relativistic regime by solving the time-dependent master equation in a multi-level model. Our ab initio approach based on the Dirac equation allows for investigating highly relativistic ions, and, consequently, provides a sensitive means to test correlated relativistic dynamics, bound-state quantum electrodynamic phenomena and nuclear effects by applying coherent light with x-ray frequencies. Atomic dipole or multipo...

  1. Spectroscopic investigation of the charge dynamics of heavy ions penetrating solid and gaseous targets

    International Nuclear Information System (INIS)

    This thesis presents the study of the slowing down process of fast heavy ions inside matter. In the framework of this research, the influence of the target density on the stopping process is investigated. Experiments on the interaction of 48Ca6+-48Ca10+ and 26Mg5+ ion beams with initial energies of 11.4 MeV/u and 5.9 MeV/u with solid and gaseous targets have been carried out. A novel diagnostic method, X-ray spectroscopy of K-shell projectile radiation, is used to determine the ion charge state in relation to its velocity during the penetration of fast heavy ions inside the stopping material. A spatially resolved analysis of the projectile and target radiation in solids is achieved for the first time. The application of low-density silica aerogels as stopping media provided a stretching of the ion stopping length by 20 - 100 times in comparison with solid quartz. The Doppler Effect observed on the projectile K-shell spectra is used to calculate the ion velocity in dependence on the ion penetration depth in the target material. A comparative analysis of Kα spectra of fast heavy ions is performed in solid (silica aerogels) and gaseous targets (Ar and Ne gases) at the same ion energy. It is shown that the dominant role of collisions in dense matter leads to an increase of the effective ionization cross section at high ion velocity and suppression of the electron capture to the projectile ion excited states at low ion velocity. As a result, an increase of the ion charge state in dense matter is observed. The experimentally detected effects are interpreted with numerical calculations of the projectile population kinetics, which are in good agreement with measurements. (orig.)

  2. Spectroscopic investigation of the charge dynamics of heavy ions penetrating solid and gaseous targets

    Energy Technology Data Exchange (ETDEWEB)

    Korostiy, S.

    2007-01-15

    This thesis presents the study of the slowing down process of fast heavy ions inside matter. In the framework of this research, the influence of the target density on the stopping process is investigated. Experiments on the interaction of {sup 48}Ca{sup 6+}-{sup 48}Ca{sup 10+} and {sup 26}Mg{sup 5+} ion beams with initial energies of 11.4 MeV/u and 5.9 MeV/u with solid and gaseous targets have been carried out. A novel diagnostic method, X-ray spectroscopy of K-shell projectile radiation, is used to determine the ion charge state in relation to its velocity during the penetration of fast heavy ions inside the stopping material. A spatially resolved analysis of the projectile and target radiation in solids is achieved for the first time. The application of low-density silica aerogels as stopping media provided a stretching of the ion stopping length by 20 - 100 times in comparison with solid quartz. The Doppler Effect observed on the projectile K-shell spectra is used to calculate the ion velocity in dependence on the ion penetration depth in the target material. A comparative analysis of K{sub {alpha}} spectra of fast heavy ions is performed in solid (silica aerogels) and gaseous targets (Ar and Ne gases) at the same ion energy. It is shown that the dominant role of collisions in dense matter leads to an increase of the effective ionization cross section at high ion velocity and suppression of the electron capture to the projectile ion excited states at low ion velocity. As a result, an increase of the ion charge state in dense matter is observed. The experimentally detected effects are interpreted with numerical calculations of the projectile population kinetics, which are in good agreement with measurements. (orig.)

  3. Characteristic X-ray radiation and Auger electrons from resonant coherently excited highly charged ions under channeling

    OpenAIRE

    Balashov, V.V.; Sokolik, A.; Stysin, A.

    2008-01-01

    Density-matrix approach to treat resonant coherent excitation of swift ions in oriented crystals is applied for unified theoretical description of charge state distribution of relativistic resonant coherently excited ions, their characteristic X-ray radiation and, as a new aspect, Auger electron production from doubly excited states.

  4. Prompt and delayed fragmentation of bromouracil cations ionized by multiply charged ions

    International Nuclear Information System (INIS)

    The fragmentation of singly and multiply charged 5-bromouracil molecules (C4H3N2O2Br) induced by collisions with slow multiply charged ions has been studied. The emission of neutral fragments as well as charge separating decay channels are identified as a function of the projectile charge state. In the first case, delayed loss of neutral moieties, occurring on a μs time scale, indicates a wider internal energy distribution resulting in a power law decay. In the second case, the most important decay channels, leading to the formation of Br+, HNCO+ and CO+/NHCH+, are discussed showing that in many processes intramolecular H-migration occurs before fragmentation. Furthermore, molecular rearrangement may lead to delayed charge separating processes. Although the dication of bromouracil is unstable, smaller doubly charged systems created by the loss of neutral fragments are found to be (meta) stable. (authors)

  5. Quantum-State-Resolved Ion-Molecule Chemistry

    Science.gov (United States)

    Chen, Gary; Yang, Tiangang; Campbell, Wesley; Hudson, Eric

    2016-05-01

    We propose a method to achieve quantum-state-resolved ion-molecule chemistry by utilizing cryogenic buffer gas cooling techniques and a combination of ion imaging and mass spectrometry of targets in an RF Paul trap. Cold molecular species produced by a cryogenic buffer gas beam (CBGB) are introduced to target ion species in an linear quadrupole trap (LQT) where ion imaging techniques and time of flight mass spectrometry (ToF) are then used to observe the target ions and the charged reaction products [1,2]. By taking advantage of the large ion-neutral interaction cross sections and characteristically long ion trap lifetimes, we can utilize the precision control over quantum states allowed by an ion trap to resolve state-to-state quantum chemical reactions without high-density molecular sample production, well within proposed capabilities. The combination of these two very general cold species production techniques allows for production and observation of a broad range of ion-neutral reactions. We initially plan to study chemical reactions between sympathetically cooled carbon ions (via laser cooled beryllium ions) with buffer gas cooled water. This work is supported by the US Air Force Office of Scientific Research.

  6. Cold highly charged ions in a cryogenic Paul trap

    DEFF Research Database (Denmark)

    Versolato, O.O.; Schwarz, M.; Windberger, A.; Ullrich, J.; Schmidt, P.O.; Drewsen, M.; Crespo López-Urrutia, J.R.

    Narrow optical transitions in highly charged ions (HCIs) are of particular interest for metrology and fundamental physics, exploiting the high sensitivity of HCIs to new physics. The highest sensitivity for a changing fine structure constant ever predicted for a stable atomic system is found in Ir...... linear Paul trap in which HCIs will be sympathetically cooled by 9Be +  ions. Optimized optical access for laser light is provided while maintaining excellent UHV conditions. The Paul trap will be connected to an electron beam ion trap (EBIT) which is able to produce a wide range of HCIs. This EBIT will...

  7. Highly charged ions generated with intense laser beams

    Czech Academy of Sciences Publication Activity Database

    Krása, Josef; Jungwirth, Karel; Králiková, Božena; Láska, Leoš; Pfeifer, Miroslav; Rohlena, Karel; Skála, Jiří; Ullschmied, Jiří; Hnatowicz, Vladimír; Peřina, Vratislav; Badziak, J.; Parys, P.; Wolowski, J.; Woryna, E.; Szydlowski, A.

    2003-01-01

    Roč. 205, - (2003), s. 355-359. ISSN 0168-583X. [International Symposium on Swift Heavy Ions in Matter /5./. Taormina-Giardini Naxos, 22.05.2002-25.05.2002] R&D Projects: GA MŠk LN00A100 Grant ostatní: HPRI(XE) CT-1999-00053; IAEA(XE) 11535/RO Institutional research plan: CEZ:AV0Z2043910; CEZ:AV0Z1010921 Keywords : laser-produced plasma * highly charged ions * ion implantation * windowless electron multiplier Subject RIV: BH - Optics, Masers, Lasers Impact factor: 1.041, year: 2003

  8. Photodetachment cross-section of the negatively charged hydrogen ion

    OpenAIRE

    Frolov, Alexei M.

    2015-01-01

    Photodetachment cross-section $\\sigma_{ph}(p_e)$ of the negatively charged hydrogen ion H$^{-}$ is determined with the use of highly accurate variational wave functions constructed for this ion. Photodetachment cross-sections of the H$^{-}$ ion are also studied for very small and very large values of the photo-electron momentum $p_e$. Maximum of this cross-section and its location have been evaluated to high accuracy. In particular, we have found that $[\\sigma_{ph}(p_e)]_{\\max} \\approx$ 3.862...

  9. On highly accurate computations of some properties of the negatively charged positronium and hydrogen ions

    OpenAIRE

    Frolov, Alexei M.

    2015-01-01

    Numerical values of some important electron-positron and electron-electron expectation values are reported for the ground (bound) $1^1S-$state of the negatively charged Ps$^{-}$ and H$^{-}$ ions. Convergence of these values upon the total number of basis functions $N$ used is briefly discussed.

  10. Systematics of Charged Particle Production in Heavy-Ion Collisions with the PHOBOS Detector at Rhic

    Science.gov (United States)

    Steinberg, Peter A.; Back, B. B.; Baker, M. D.; Barton, D. S.; Betts, R. R.; Bindel, R.; Budzanowski, A.; Busza, W.; Carroll, A.; Corbo, J.; Decowski, M. P.; Garcia, E.; George, N.; Gulbrandsen, K.; Gushue, S.; Halliwell, C.; Hamblen, J.; Henderson, C.; Hicks, D.; Hofman, D.; Hollis, R. S.; Hołyński, R.; Holzman, B.; Iordanova, A.; Johnson, E.; Kane, J.; Katzy, J.; Khan, N.; Kucewicz, W.; Kulinich, P.; Kuo, C. M.; Lin, W. T.; Manly, S.; McLeod, D.; Michałowski, J.; Mignerey, A.; Mülmenstädt, J.; Nouicer, R.; Olszewski, A.; Pak, R.; Park, I. C.; Pernegger, H.; Rafelski, M.; Rbeiz, M.; Reed, C.; Remsberg, L. P.; Reuter, M.; Roland, C.; Roland, G.; Rosenberg, L.; Sagerer, J.; Sarin, P.; Sawicki, P.; Skulski, W.; Steadman, S. G.; Steinberg, P.; Stephans, G. S. F.; Stodulski, M.; Sukhanov, A.; Tang, J.-L.; Teng, R.; Trzupek, A.; Vale, C.; van Nieuwenhuizen, G. J.; Verdier, R.; Wadsworth, B.; Wolfs, F. L. H.; Wosiek, B.; Woźniak, K.; Wuosmaa, A. H.; Wysłouch, B.

    2002-03-01

    The multiplicity of charged particles produced in Au+Au collisions as a function of energy, centrality, rapidity and azimuthal angle has been measured with the PHOBOS detector at RHIC. These results contribute to our understanding of the initial state of heavy ion collisions and provide a means to compare basic features of particle production in nuclear collisions with more elementary systems.

  11. Photodissociation and charge transfer dynamics of negative ions studied with femtosecond photoelectron spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Zanni, Martin T.

    1999-12-17

    This dissertation presents studies aimed at understanding the potential energy surfaces and dynamics of isolated negative ions, and the effects of solvent on each. Although negative ions play important roles in atmospheric and solution phase chemistry, to a large extent the ground and excited state potential energy surfaces of gas phase negative ions are poorly characterized, and solvent effects even less well understood. In an effort to fill this gap, the author's coworkers and the author have developed a new technique, anion femtosecond photoelectron spectroscopy, and applied it to gas phase photodissociation and charge transfer processes. Studies are presented that (1) characterize the ground and excited states of isolated and clustered anions, (2) monitor the photodissociation dynamics of isolated and clustered anions, and (3) explore the charge-transfer-to-solvent states of atomic iodide clustered with polar and non-polar solvents.

  12. Photodissociation and charge transfer dynamics of negative ions studied with femtosecond photoelectron spectroscopy

    International Nuclear Information System (INIS)

    This dissertation presents studies aimed at understanding the potential energy surfaces and dynamics of isolated negative ions, and the effects of solvent on each. Although negative ions play important roles in atmospheric and solution phase chemistry, to a large extent the ground and excited state potential energy surfaces of gas phase negative ions are poorly characterized, and solvent effects even less well understood. In an effort to fill this gap, the author's coworkers and the author have developed a new technique, anion femtosecond photoelectron spectroscopy, and applied it to gas phase photodissociation and charge transfer processes. Studies are presented that (1) characterize the ground and excited states of isolated and clustered anions, (2) monitor the photodissociation dynamics of isolated and clustered anions, and (3) explore the charge-transfer-to-solvent states of atomic iodide clustered with polar and non-polar solvents

  13. Numerical calculation of impurity charge state distributions

    Energy Technology Data Exchange (ETDEWEB)

    Crume, E. C.; Arnurius, D. E.

    1977-09-01

    The numerical calculation of impurity charge state distributions using the computer program IMPDYN is discussed. The time-dependent corona atomic physics model used in the calculations is reviewed, and general and specific treatments of electron impact ionization and recombination are referenced. The complete program and two examples relating to tokamak plasmas are given on a microfiche so that a user may verify that his version of the program is working properly. In the discussion of the examples, the corona steady-state approximation is shown to have significant defects when the plasma environment, particularly the electron temperature, is changing rapidly.

  14. Production of highly charged ions of argon by optical field ionization in a relativistic laser field

    International Nuclear Information System (INIS)

    We observed the highly charged ions of argon by optical field ionization in a relativistic intensity regime. Charge states up to Ar15+ were produced at the highest intensity of 800 nm, linearly polarized 20 fs Ti: sapphire laser pulses. The peak intensity of the pulse is determined by comparing the measured ion production curve for Ar9+ with ADK theory. The results of these measurements of the ionization indicate that the maximum peak intensity is achieved to ∼2x1019 W/cm2. (author)

  15. Technique of Producing High Charge State Heavy-ion Beam%高电荷态重离子束流产生技术的研究

    Institute of Scientific and Technical Information of China (English)

    高丽娟; 范辉; 蔡莉; 王惠; 史淑廷; 郭刚; 刘建成; 陈泉; 沈东军; 惠宁; 王贵良; 孔福全

    2014-01-01

    为了提高北京HI-13串列加速器束流的硅中射程和LET 值,本文开展了高电荷态束流引出技术及pA级弱束流诊断技术研究。采用电刚度和磁刚度模拟技术,配合pA级弱束流束斑观测和束流强度监测技术,获得能量360 MeV、峰总比80%的197 Au离子束流,其在Si中的表面LET为86.1 MeV · cm2· mg -1、射程为30.1μm ,满足单粒子效应(SEE)实验的要求,拓展了北京 HI-13串列加速器上单粒子效应实验所用离子的能量和LET值范围。%In order to get the Beijing HI-13 tandem accelerator beam with the higher range and LET in silicon , the techniques of beam route simulating and pico-ampere beam diagnosing were developed .The magnetic rigidity simulation and electric rigidity simulation techniques combined with beam spot observing and beam intensity measuring techniques were used for getting 360 MeV 197 Au ion beam with the peak-to-total ratio of 80% in the spectrum .The range of 360 MeV 197 Au in silicon is 30.1μm and the LET is 86.1 MeV · cm2 · mg -1 .This meets the requirement of single-event effect test ,and the beam energy range and LET range in Beijing HI-13 tandem accelerator have been obvi-ously enlarged .

  16. 高电荷态重离子束流产生技术的研究%Technique of Producing High Charge State Heavy-ion Beam

    Institute of Scientific and Technical Information of China (English)

    高丽娟; 范辉; 蔡莉; 王惠; 史淑廷; 郭刚; 刘建成; 陈泉; 沈东军; 惠宁; 王贵良; 孔福全

    2014-01-01

    In order to get the Beijing HI-13 tandem accelerator beam with the higher range and LET in silicon , the techniques of beam route simulating and pico-ampere beam diagnosing were developed .The magnetic rigidity simulation and electric rigidity simulation techniques combined with beam spot observing and beam intensity measuring techniques were used for getting 360 MeV 197 Au ion beam with the peak-to-total ratio of 80% in the spectrum .The range of 360 MeV 197 Au in silicon is 30.1μm and the LET is 86.1 MeV · cm2 · mg -1 .This meets the requirement of single-event effect test ,and the beam energy range and LET range in Beijing HI-13 tandem accelerator have been obvi-ously enlarged .%为了提高北京HI-13串列加速器束流的硅中射程和LET 值,本文开展了高电荷态束流引出技术及pA级弱束流诊断技术研究。采用电刚度和磁刚度模拟技术,配合pA级弱束流束斑观测和束流强度监测技术,获得能量360 MeV、峰总比80%的197 Au离子束流,其在Si中的表面LET为86.1 MeV · cm2· mg -1、射程为30.1μm ,满足单粒子效应(SEE)实验的要求,拓展了北京 HI-13串列加速器上单粒子效应实验所用离子的能量和LET值范围。

  17. Charge exchange spectroscopy as a fast ion diagnostic on TEXTOR

    NARCIS (Netherlands)

    Delabie, E.; Jaspers, R. J. E.; von Hellermann, M. G.; Nielsen, S.K.; Marchuk, O.

    2008-01-01

    An upgraded charge exchange spectroscopy diagnostic has been taken into operation at the TEXTOR tokamak. The angles of the viewing lines with the toroidal magnetic field are close to the pitch angles at birth of fast ions injected by one of the neutral beam injectors. Using another neutral beam for

  18. Collisions of slow highly charged ions with surfaces

    OpenAIRE

    Burgdoerfer, J.; Lemell, C.; Schiessl, K.; Solleder, B.; Reinhold, C.; Tokesi, K.; Wirtz, Ludger

    2006-01-01

    Progress in the study of collisions of multiply charged ions with surfaces is reviewed with the help of a few recent examples. They range from fundamental quasi-one electron processes to highly complex ablation and material modification processes. Open questions and possible future directions will be discussed.

  19. Charge exchange emission from solar wind helium ions

    NARCIS (Netherlands)

    Bodewits, D; Hoekstra, R; Seredyuk, B; McCullough, RW; Jones, GH; Tielens, AGGM

    2006-01-01

    Charge exchange X-ray and far-ultraviolet (FUV) aurorae can provide detailed insight into the interaction between solar system plasmas. Using the two complementary experimental techniques of photon emission spectroscopy and translation energy spectroscopy, we have studied state-selective charge exch

  20. Charge breeding results and future prospects with electron cyclotron resonance ion source and electron beam ion source (invited).

    Science.gov (United States)

    Vondrasek, R; Levand, A; Pardo, R; Savard, G; Scott, R

    2012-02-01

    The Californium Rare Ion Breeder Upgrade (CARIBU) of the Argonne National Laboratory ATLAS facility will provide low-energy and reaccelerated neutron-rich radioactive beams for the nuclear physics program. A 70 mCi (252)Cf source produces fission fragments which are thermalized and collected by a helium gas catcher into a low-energy particle beam with a charge of 1+ or 2+. An electron cyclotron resonance (ECR) ion source functions as a charge breeder in order to raise the ion charge sufficiently for acceleration in the ATLAS linac. The final CARIBU configuration will utilize a 1 Ci (252)Cf source to produce radioactive beams with intensities up to 10(6) ions∕s for use in the ATLAS facility. The ECR charge breeder has been tested with stable beam injection and has achieved charge breeding efficiencies of 3.6% for (23)Na(8+), 15.6% for (84)Kr(17+), and 13.7% for (85)Rb(19+) with typical breeding times of 10 ms∕charge state. For the first radioactive beams, a charge breeding efficiency of 11.7% has been achieved for (143)Cs(27+) and 14.7% for (143)Ba(27+). The project has been commissioned with a radioactive beam of (143)Ba(27+) accelerated to 6.1 MeV∕u. In order to take advantage of its lower residual contamination, an EBIS charge breeder will replace the ECR charge breeder in the next two years. The advantages and disadvantages of the two techniques are compared taking into account the requirements of the next generation radioactive beam facilities. PMID:22380254

  1. P.I.A.F.E. project: production of highly charged particles for radioactive ion beams

    International Nuclear Information System (INIS)

    The transformation of a mono-charged ion beam into a multicharged ion beam is an important problem in the projects of radioactive beams acceleration. This transformation must be performed with the best possible efficiency and in the shortest possible time to avoid the loss of particles by radioactive degenerescence. A ionization method using an electron cyclotron resonance (ECR) source is proposed. It consists in the fast capture by the ECR plasma of the radioactive elements injected inside this source in the form of a mono-charged ion beam. This method gives good results (2 to 6% efficiency to move from the 1+ to the 9+ charge state) for the ionization of alkaline elements, rare and metallic gases, with fast times of response allowing the ionization of radioactive products with a lifetime inferior to 1 s. (J.S.)

  2. Determination of the charge state distribution of a highly ionized coronal Au plasma

    International Nuclear Information System (INIS)

    We present the first definitive measurement of the charge state distribution of a highly ionized gold plasma in coronal equilibrium. The experiment utilized the Livermore electron beam ion trap EBIT-II in a novel configuration to create a plasma with a Maxwellian temperature of 2.5 keV. The charge balance in the plasma was inferred from spectral line emission measurements which accounted for charge exchange effects. The measured average ionization state was 46.8±0.75. This differs from the predictions of two modeling codes by up to four charge states

  3. State approaches to the system benefits charge

    Energy Technology Data Exchange (ETDEWEB)

    Fang, J M

    1997-07-01

    This report documents the consideration and implementation of a non-bypassable system benefits charge (SBC) in six states through mid-May 1997. The SBC is being established to sustain important public-policy programs during the electric industry restructuring process. The states covered include Arizona, California, Massachusetts, New York, Rhode Island, and Wisconsin. This report was prepared for the Office of Energy and Resource Planning, Utah Department of Natural Resources, under the National Renewable Energy Laboratory`s Sustainable Technology Energy Partnerships Initiative, Second Round (STEP-2). The purpose of the report is to provide decision makers in Utah, including the Utah Public Service Commission and the state legislature, with relevant information on the SBC for use in their deliberation on the matter. The issues faced by the six states are the SBC in general; surcharge rate or funding levels; administrative structure and procedures; and actions, guidelines, and principles by program area.

  4. Testing double ionization mechanisms with highly-charged ions

    International Nuclear Information System (INIS)

    Double ionization of He target atoms by intermediate- to high-velocity charged ions is considered in terms of two mechanisms: (1) a two-step (TS) process in which both target electrons are removed in separate direct interactions with the projectile, and (2) a one-step mechanism in which one electron is liberated in a single projectile-target interaction followed by subsequent ''shakeoff'' (SO) of the second electron. Measured double-to-single ionization ratios are used to exhibit and test the underlying mechanisms of double ionization. It is found that these ratios exhibit a high degree of universality as a function of v/q, where v is the velocity of the ion and q is its charge. The results strongly suggest that the important factor in determining the regions of validity for TS and SO is the ionic charge divided by the impact velocity and not just the impact velocity itself

  5. Magnetohydrodynamics and charge identified directed flow in heavy ion collisions

    Science.gov (United States)

    Gürsoy, Umut; Kharzeev, Dmitri; Rajagopal, Krishna

    2016-01-01

    Strong magnetic fields produced in any non-central heavy ion collision are expected to affect the dynamics of the hot QCD matter produced in this collision. The magnetic field is time-dependent and the medium is expanding, which leads to the induction of charged currents due to the combination of Faraday and Hall effects. We study the imprint the magnetic fields produced in non-central heavy ion collisions leave on the azimuthal distributions and correlations of the produced charged hadrons by employing an analytic solution to hydrodynamics combined with the electromagnetic effects in a perturbative fashion. We use the Cooper-Frye freeze-out procedure on an isothermal freeze-out surface to obtain the azimuthal hadron distributions. We find that the charged currents induced by the present of the electromagnetic fields result in a charge-dependent directed flow v1 that is odd in rapidity and odd under charge exchange. It can be detected by measuring correlations between the directed flow of charged hadrons at different rapidities, .

  6. High resolution charge spectroscopy of heavy ions with FNTD technology

    International Nuclear Information System (INIS)

    Highlights: •FNTD technology was utilized to obtain charge spectra of carbon-ion fragments. •Several correction techniques were developed to minimize line broadening. •Charge resolution of 0.25 c.u. was demonstrated. •Light fragments starting from hydrogen and helium were detected. -- Abstract: This paper is focused on the improvement of the heavy charge particle charge resolution of Fluorescent Nuclear Track Detector (FNTD) technology. Fluorescent intensity of individual heavy charge particle tracks is used to construct the spectrum. Sources of spectroscopic line broadening were investigated and several fluorescent intensity correction procedures were introduced to improve the charge resolution down to δZ = 0.25 c.u. and enable FNTD technology to distinguish between all projectile fragments of 290 MeV carbon ions. The benefits of using FNTD technology for fragmentation study include large dynamic range and wide angular acceptance. While we describe these developments in the context of fragmentation studies, the same techniques are readily extended to FNTD LET spectroscopy in general

  7. Negative ion-uranium hexafluoride charge transfer reactions

    Science.gov (United States)

    Streit, Gerald E.; Newton, T. W.

    1980-10-01

    The flowing afterglow technique has been used to study the process of charge transfer from selected negative ions (F-, Cl-, Br-, I-, SF6-) to UF6. The sole ionic product in all cases was observed to be UF6-. Data analysis was complicated by an unexpected coupling of chemical and diffusive ion loss processes when UF6- product ions were present. The rate coefficients for the charge transfer processes are (k in 10-9 cm3 molecule-1 s-1) F-, 1.3; Cl-, 1.1; Br-, 0.93; I-, 0.77; and SF6-, 0.69. The rate constants agree quite well with the classical Langevin predictions.

  8. Contribution of charge-transfer processes to ion-induced electron emission

    International Nuclear Information System (INIS)

    Charge changing events of ions moving inside metals are shown to contribute significantly to electron emission in the intermediate velocity regime via electrons coming from projectile ionization. Inclusion of equilibrium charge state fractions, together with two-electron Auger processes and resonant-coherent electron loss from the projectile, results in reasonable agreement with previous calculations for frozen protons, though a significant part of the emission is now interpreted in terms of charge exchange. The quantal character of the surface barrier transmission is shown to play an important role. The theory compares well with experimental observations for H projectiles. copyright 1996 The American Physical Society

  9. Contribution of charge-transfer processes to ion-induced electron emission

    Energy Technology Data Exchange (ETDEWEB)

    Roesler, M. [Departamento de Fisica de Materiales, Facultad de Quimica, UPV/EHU, Apartado 1072, 20080 San Sebastian (Spain); Garcia de Abajo, F.J. [Departamento de Ciencias de la Computacion e Inteligencia Artificial, Facultad de Informatica, UPV/EHU, Apartado 649, 20080 San Sebastian (Spain)

    1996-12-01

    Charge changing events of ions moving inside metals are shown to contribute significantly to electron emission in the intermediate velocity regime via electrons coming from projectile ionization. Inclusion of equilibrium charge state fractions, together with two-electron Auger processes and resonant-coherent electron loss from the projectile, results in reasonable agreement with previous calculations for frozen protons, though a significant part of the emission is now interpreted in terms of charge exchange. The quantal character of the surface barrier transmission is shown to play an important role. The theory compares well with experimental observations for {ital H} projectiles. {copyright} {ital 1996 The American Physical Society.}

  10. Supercharging with m-nitrobenzyl alcohol and propylene carbonate: forming highly charged ions with extended, near-linear conformations.

    Science.gov (United States)

    Going, Catherine C; Williams, Evan R

    2015-04-01

    The effectiveness of the supercharging reagents m-nitrobenzyl alcohol (m-NBA) and propylene carbonate at producing highly charged protein ions in electrospray ionization is compared. Addition of 5% m-NBA or 15% propylene carbonate increases the average charge of three proteins by ∼21% or ∼23%, respectively, when these ions are formed from denaturing solutions (water/methanol/acetic acid). These results indicate that both reagents are nearly equally effective at supercharging when used at their optimum concentrations. A narrowing of the charge state distribution occurs with both reagents, although this effect is greater for propylene carbonate. Focusing the ion signal into fewer charge states has the advantage of improving sensitivity. The maximum charge state of ubiquitin formed with propylene carbonate is 21+, four charges higher than previously reported. Up to nearly 30% of all residues in a protein can be charged, and the collisional cross sections of the most highly charged ions of both ubiquitin and cytochrome c formed with these supercharging reagents were measured for the first time and found to be similar to those calculated for theoretical highly extended, linear or near-linear conformations. Under native supercharging conditions, m-NBA is significantly more effective at producing high charge states than propylene carbonate. PMID:25719488

  11. Influence of charge changing collisions on charge state distributions (CSD) in non-equilibrium plasmas

    International Nuclear Information System (INIS)

    For an optimal design of ion sources and for some aspects of plasma diagnostics it is important to study the influence of all processes and parameters that are essential for the production and loss of multiply charged ions. Till now all existing calculations of CSD neglected charge transfer because of missing data. Now many of the very big charge transfer cross sections are measured and so we are able to include them into our calculations. (orig.)

  12. SMILETRAP - A Penning trap facility for precision mass measurements using highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Bergstroem, I.; Carlberg, C.; Fritioff, T.; Douysset, G.; Schoenfelder, J.; Schuch, R. E-mail: schuch@physto.se

    2002-07-21

    The precision of mass measurements in a Penning trap increases linearly with the charge of the ion. Therefore we have attached a Penning trap, named SMILETRAP, to the electron beam ion source CRYSIS at MSL. CRYSIS is via an isotope separator connected to an ion source that can deliver singly charged ions of practically any element. In CRYSIS charge state breeding occurs by intense electron bombardment. We have shown that it is possible to produce, catch and measure the cyclotron frequencies of ions in the charge region 1+ to 52+. The relevant observable in mass measurements using a Penning trap is the ratio of the cyclotron frequencies of the ion of interest and ion used as a mass reference. High precision requires that the two frequencies are measured after one another in the shortest possible time. For reasons of convenience the precision trap operates at room temperature. So far it has been believed that warm traps working at 4 K are required for high mass precision with exactly one ion in the trap at a time. In this paper we demonstrate that mass precision of a few parts in 10{sup 10} also can be obtained in a warm trap at a pressure of about 5x10{sup -12} mbar by stabilizing the pressure in the He-dewar, the trap temperature and the frequency synthesizer. In order to reduce the influence of changes of the magnetic field to a level below 10{sup -10}, the scanning of the frequencies close to the resonances of both the ion of interest and the reference ion is done in a total time <2 min. Trapping of ions is a statistical procedure, allowing more than one ion to be trapped in each measurement cycle. However, after completing the measurements it is possible to reject all information except for events based on 1 and 2 trapped ions. The procedures of producing, transporting, catching, exciting and measuring the cyclotron resonance frequencies of highly charged ions and the mass reference ions with the time-of-flight method are described. In routine measurements with

  13. Experimental study of interactions of highly charged ions with atoms at keV energies: Progress report for period May 15, 1985-February 15, 1987

    International Nuclear Information System (INIS)

    Interest in interactions of low energy highly charged ions with electrons, atoms or ions is due to their importance to controlled thermonuclear fusion research and the interesting nature of the fundamental processes involved. Studies of such interactions have long been hampered by a lack of suitable ions sources. A superconducting solenoid, cryogenic Electron Beam Ion Source, CEBIS, has been constructed at Cornell University to produce low energy very highly charged ions. At present, using a pulsed 0.5A,8.5 keV electron beam, the source is capable of producing highly charged ions of C,N,O, including bare nuclei, and ions of Ar up to charge state 11 + in 1 millisecond of confinement time. The source is being used in experiments to investigate charge transfer and accompanying processes in low energy, highly charged ion-atom collisions

  14. Photo-induced changes in charge-ordered state of Ti4O7

    International Nuclear Information System (INIS)

    We have investigated photo-induced effects on the charge-ordered state of Ti4O7 with pump-probe spectroscopy. Reflectivity of the probe light changes after the pulsed pump excitation, and then recovers. The photo-induced effects are observed only when the pump power exceeds a threshold value, indicative of cooperative nature of the formation process, and the recovery rate shows thermally activated behaviour. We propose that the photo-induced state is a metastable charge localized state where charge disorder is induced by a photon-assisted charge transfer process from Ti26+ dimers to the neighbouring Ti4+ions. Moreover, it is found that subsequent cw laser irradiation converts the photo-induced state into the charge-ordered state. We interpret this result in terms of formation of Ti26+ dimers via an inverse charge transfer process assisted by the cw optical excitation.

  15. High resolution charge spectroscopy of heavy ions with FNTD technology

    Science.gov (United States)

    Bartz, J. A.; Kodaira, S.; Kurano, M.; Yasuda, N.; Akselrod, M. S.

    2014-09-01

    This paper is focused on the improvement of the heavy charge particle charge resolution of Fluorescent Nuclear Track Detector (FNTD) technology. Fluorescent intensity of individual heavy charge particle tracks is used to construct the spectrum. Sources of spectroscopic line broadening were investigated and several fluorescent intensity correction procedures were introduced to improve the charge resolution down to δZ = 0.25 c.u. and enable FNTD technology to distinguish between all projectile fragments of 290 MeV carbon ions. The benefits of using FNTD technology for fragmentation study include large dynamic range and wide angular acceptance. While we describe these developments in the context of fragmentation studies, the same techniques are readily extended to FNTD LET spectroscopy in general.

  16. Properties of cold ions produced by synchrotron radiation and by charged particle impact

    International Nuclear Information System (INIS)

    Argon recoil ions produced by beams of 0.8 MeV/u Cl5+ have been detected by time-of-flight (TOF) techniques in coincidence with the loss of from one to five projectile electrons. Recoil-ion energies have been determined to be more than an order of magnitude higher than those of highly-charged ions produced by unmonochromatized synchrotron radiation. Charge-state distributions, however, show similarities, suggesting that loss of projectile electrons corresponds, in some cases, to inner-shell target ionization producing vacancy cascades. In an essential improvement to the usual multinomial description of ionization in the independent-electron-ejection model, we find the inclusion of Auger vacancy cascades significantly alters the description of the recoil ion spectra corresponding to projectile-electron loss. These conclusions are consistent with impact parameters inferred from determinations of mean recoil energy. 11 refs., 5 figs

  17. Properties of cold ions produced by synchrotron radiation and by charged particle impact

    International Nuclear Information System (INIS)

    Argon recoil ions produced by beams of 0.8 MeV/u Cl5+ have been detected by time-of-flight (TOF) techniques in coincidence with the loss of from one to five projectile electrons. Recoil-ion energies have been determined to be more than an order of magnitude higher than those of highly charged ions poduced by unmonochromatized synchrotron radiation. Charge-state distributions, however, show similarities, suggesting that loss of projectile electrons corresponds, in some cases, to inner-shell target ionization producing vacancy cascades. In an essential improvement to the usual multinomial description of ionization in the dependent-electron-ejection model, we find the inclusion Auger vacancy cascades significantly alters the description of the recoil ion spectra corresponding to the projectile-electron loss. These conclusions are consistent with impact parameters inferred from determination of mean recoil energy. (orig.)

  18. Charge collection efficiency degradation induced by MeV ions in semiconductor devices: Model and experiment

    Science.gov (United States)

    Vittone, E.; Pastuovic, Z.; Breese, M. B. H.; Garcia Lopez, J.; Jaksic, M.; Raisanen, J.; Siegele, R.; Simon, A.; Vizkelethy, G.

    2016-04-01

    This paper investigates both theoretically and experimentally the charge collection efficiency (CCE) degradation in silicon diodes induced by energetic ions. Ion Beam Induced Charge (IBIC) measurements carried out on n- and p-type silicon diodes which were previously irradiated with MeV He ions show evidence that the CCE degradation does not only depend on the mass, energy and fluence of the damaging ion, but also depends on the ion probe species and on the polarization state of the device. A general one-dimensional model is derived, which accounts for the ion-induced defect distribution, the ionization profile of the probing ion and the charge induction mechanism. Using the ionizing and non-ionizing energy loss profiles resulting from simulations based on the binary collision approximation and on the electrostatic/transport parameters of the diode under study as input, the model is able to accurately reproduce the experimental CCE degradation curves without introducing any phenomenological additional term or formula. Although limited to low level of damage, the model is quite general, including the displacement damage approach as a special case and can be applied to any semiconductor device. It provides a method to measure the capture coefficients of the radiation induced recombination centres. They can be considered indexes, which can contribute to assessing the relative radiation hardness of semiconductor materials.

  19. Proceedings of the workshop on opportunities for atomic physics using slow, highly-charged ions

    International Nuclear Information System (INIS)

    The study of atomic physics with highly-charged ions is an area of intense activity at the present time because of a convergence of theoretical interest and advances in experimental techniques. The purpose of the Argonne ''Workshop on Opportunities for Atomic Physics Using Slow, Highly-Charged Ions'' was to bring together atomic, nuclear, and accelerator physicists in order to identify what new facilities would be most useful for the atomic physics community. The program included discussion of existing once-through machines, advanced ion sources, recoil ion techniques, ion traps, and cooler rings. One of the topics of the Workshop was to discuss possible improvement to the ANL Tandem-Linac facility (ATLAS) to enhance the capability for slowing down ions after they are stripped to a high-charge state (the Accel/Decel technique). Another topic was the opportunity for atomic physics provided by the ECR ion source which is being built for the Uranium Upgrade of ATLAS. 18 analytics were prepared for the individual papers in this volume

  20. Proceedings of the workshop on opportunities for atomic physics using slow, highly-charged ions

    Energy Technology Data Exchange (ETDEWEB)

    1987-01-01

    The study of atomic physics with highly-charged ions is an area of intense activity at the present time because of a convergence of theoretical interest and advances in experimental techniques. The purpose of the Argonne ''Workshop on Opportunities for Atomic Physics Using Slow, Highly-Charged Ions'' was to bring together atomic, nuclear, and accelerator physicists in order to identify what new facilities would be most useful for the atomic physics community. The program included discussion of existing once-through machines, advanced ion sources, recoil ion techniques, ion traps, and cooler rings. One of the topics of the Workshop was to discuss possible improvement to the ANL Tandem-Linac facility (ATLAS) to enhance the capability for slowing down ions after they are stripped to a high-charge state (the Accel/Decel technique). Another topic was the opportunity for atomic physics provided by the ECR ion source which is being built for the Uranium Upgrade of ATLAS. 18 analytics were prepared for the individual papers in this volume.

  1. Study on space charge effect in an electrostatic ion analyzer applied to measure laser produced ions

    International Nuclear Information System (INIS)

    The abundance of different ions produced by laser ion sources is usually analyzed by an electrostatic ion analyzer (EIA). Ion current intensities in the range of several mA/cm2 at the position of the EIA have been achieved from the laser ion source developed by the Institute of Modern Physics; this indicates that a noticeable influence of space charge effect during the ion transmission will occur. Hence, while the parameters of the EIA or the beams are changed, such as ion species, current intensity, the ions’ transmission efficiency through the EIA is different, which will result in an uncertainty in the estimation of the ions’ yields. Special attention is focused on this issue in this paper. Ion's transmissions through the EIA under different circumstances are studied with simulations and experiments, the results of which are consistent with each other

  2. Charge exchange spectroscopy as a fast ion diagnostic on TEXTOR

    DEFF Research Database (Denmark)

    Delabie, E.; Jaspers, R.J.E.; von Hellermann, M.G.;

    2008-01-01

    active spectroscopy, injected counter the direction in which fast ions injected by the first beam are circulating, we can simultaneously measure a fast ion tail on the blue wing of the D-alpha spectrum while the beam emission spectrum is Doppler shifted to the red wing. An analysis combining the two......An upgraded charge exchange spectroscopy diagnostic has been taken into operation at the TEXTOR tokamak. The angles of the viewing lines with the toroidal magnetic field are close to the pitch angles at birth of fast ions injected by one of the neutral beam injectors. Using another neutral beam for...... parts of the spectrum offers possibilities to improve the accuracy of the absolute (fast) ion density profiles. Fast beam modulation or passive viewing lines cannot be used for background subtraction on this diagnostic setup and therefore the background has to be modeled and fitted to the data together...

  3. Highly charged ions at rest: The HITRAP project at GSI

    International Nuclear Information System (INIS)

    A decelerator will be installed at GSI in order to provide and study bare heavy nuclei or heavy nuclei with only few electrons at very low energies or even at rest. Highly-charged ions will be produced by stripping at relativistic energies. After electron cooling and deceleration in the Experimental Storage Ring the ions are ejected out of the storage ring at 4 MeV/u and further decelerated in a combination of an IH and RFQ structure. Finally, they are injected into a Penning trap where the ions are cooled to 4 K. From here, the ions can be transferred in a quasi dc or in a pulsed mode to different experimental setups. This article describes the technical concepts of this project as well as planned key experiments

  4. Photodetachment cross-section of the negatively charged hydrogen ion

    CERN Document Server

    Frolov, Alexei M

    2015-01-01

    Photodetachment cross-section $\\sigma_{ph}(p_e)$ of the negatively charged hydrogen ion H$^{-}$ is determined with the use of highly accurate variational wave functions constructed for this ion. Photodetachment cross-sections of the H$^{-}$ ion are also studied for very small and very large values of the photo-electron momentum $p_e$. Maximum of this cross-section has been evaluated to very high accuracy and we have found that $[\\sigma_{ph}(p_e)]_{\\max} \\approx$ 3.8627035742 $\\cdot 10^{-17}$ $cm^2$ at $p_e \\approx$ 0.113206(1) $a.u.$ Photodetachment of the H$^{-}$ ion at very small and very large $p_e$ values is also considered. Our method is based upon the Rayleigh's formula for spherical Bessel functions.

  5. Charge state and incident energy dependence of K X-ray emission as a function of target thickness for 50-165 MeV Cu ions incident on 11-250 μg/cm 2 Cu

    Science.gov (United States)

    Momoi, T.; Shima, K.; Umetani, K.; Moriyama, M.; Ishihara, T.; Mikumo, T.

    1986-05-01

    Thin self-supporting Cu targets in 11-250 μg/cm 2 thickness were bombarded with 50-165 MeV Cu qi+ ions (7 ⩽ qi⩽ 24) to investigate the target thickness dependence of inner shell vacancy production processes in the symmetric collision of Cu + Cu. Doppler-shifted projectile K X-rays were discriminated from the target K X-rays, and the projectile and target K X-ray yields were separately measured as a function of target thickness. The K X-ray yields emitted from the projectile and the target Cu atoms are strongly dependent on the projectile initial charge state and target thickness for all the investigated collision systems of Cu qi+ + Cu. From the observed K X-ray yields, K-shell vacancy production cross sections averaged over the target thickness t of projectile overlineσ KV and target overlineσ ∗KV were separately derived taking into account the fluorescence yield that can be estimated from the Kα X-ray energy shift. When the values of overlineσ KV and overlineσ ∗KV are extrapolated to zero foil thickness, the K shell vacancy formed in the collision has been found to be equally shared between projectile and target in a single collision. With the increase of penetration depth, however, the values of overlineσ ∗KV are greater than those of overlineσ KV presumably due to electron transfer of a target K electron to the projectile K vacancy. the evolution process of projectile excited states as a function of target thickness and the resulting variation of projectile and target K X-ray emissions are discussed.

  6. State of charge monitoring methods for vanadium redox flow battery control

    Science.gov (United States)

    Skyllas-Kazacos, Maria; Kazacos, Michael

    2011-10-01

    During operation of redox flow batteries, differential transfer of ions and electrolyte across the membrane and gassing side reactions during charging, can lead to an imbalance between the two half-cells that results in loss of capacity. This capacity loss can be corrected by either simple remixing of the two solutions, or by chemical or electrochemical rebalancing. In order to develop automated electrolyte management systems therefore, the state-of-charge of each half-cell electrolyte needs to be known. In this study, two state-of-charge monitoring methods are investigated for use in the vanadium redox flow battery. The first method utilizes conductivity measurements to independently measure the state-of-charge of each half-cell electrolyte. The second method is based on spectrophotometric principles and uses the different colours of the charged and discharged anolyte and catholyte to monitor system balance and state-of charge of each half-cell of the VRB during operation.

  7. Evidence of double layer/capacitive charging in carbon nanomaterial-based solid contact polymeric ion-selective electrodes.

    Science.gov (United States)

    Cuartero, Maria; Bishop, Josiah; Walker, Raymart; Acres, Robert G; Bakker, Eric; De Marco, Roland; Crespo, Gaston A

    2016-08-11

    This paper presents the first direct spectroscopic evidence for double layer or capacitive charging of carbon nanomaterial-based solid contacts in all-solid-state polymeric ion-selective electrodes (ISEs). Here, we used synchrotron radiation-X-ray photoelectron spectroscopy (SR-XPS) and SR valence band (VB) spectroscopy in the elucidation of the charging mechanism of the SCs. PMID:27405722

  8. Molecular ion battery: a rechargeable system without using any elemental ions as a charge carrier

    Science.gov (United States)

    Yao, Masaru; Sano, Hikaru; Ando, Hisanori; Kiyobayashi, Tetsu

    2015-06-01

    Is it possible to exceed the lithium redox potential in electrochemical systems? It seems impossible to exceed the lithium potential because the redox potential of the elemental lithium is the lowest among all the elements, which contributes to the high voltage characteristics of the widely used lithium ion battery. However, it should be possible when we use a molecule-based ion which is not reduced even at the lithium potential in principle. Here we propose a new model system using a molecular electrolyte salt with polymer-based active materials in order to verify whether a molecular ion species serves as a charge carrier. Although the potential of the negative-electrode is not yet lower than that of lithium at present, this study reveals that a molecular ion can work as a charge carrier in a battery and the system is certainly a molecular ion-based “rocking chair” type battery.

  9. Single ion induced surface nanostructures: a comparison between slow highly charged and swift heavy ions.

    Science.gov (United States)

    Aumayr, Friedrich; Facsko, Stefan; El-Said, Ayman S; Trautmann, Christina; Schleberger, Marika

    2011-10-01

    This topical review focuses on recent advances in the understanding of the formation of surface nanostructures, an intriguing phenomenon in ion-surface interaction due to the impact of individual ions. In many solid targets, swift heavy ions produce narrow cylindrical tracks accompanied by the formation of a surface nanostructure. More recently, a similar nanometric surface effect has been revealed for the impact of individual, very slow but highly charged ions. While swift ions transfer their large kinetic energy to the target via ionization and electronic excitation processes (electronic stopping), slow highly charged ions produce surface structures due to potential energy deposited at the top surface layers. Despite the differences in primary excitation, the similarity between the nanostructures is striking and strongly points to a common mechanism related to the energy transfer from the electronic to the lattice system of the target. A comparison of surface structures induced by swift heavy ions and slow highly charged ions provides a valuable insight to better understand the formation mechanisms. PMID:21900733

  10. Influence of Multiple Ionization on Charge State Distributions

    Science.gov (United States)

    Hahn, Michael; Savin, Daniel Wolf

    2015-08-01

    The spectrum emitted by a plasma depends on the charge state distribution (CSD) of the gas. For collisionally ionized plasmas, the CSD is is determined by the corresponding rates for electron-impact ionization and recombination. In astrophysics, such plasmas are formed in stars, supernova remnants, galaxies, and galaxy clusters. Current CSD calculations generally do not account for electron-impact multiple ionization (EIMI), a process in which multiple electrons are ejected by a single electron-ion collision. We have estimated the EIMI cross sections for all charge states of iron using a combination of the available experimental data and semi-empirical formulae. We then modeled the CSD and observed the influence of EIMI compared to only including single ionization. One case of interest for astrophysics is nanoflare heating, which is a leading theory to explain the heating of the solar corona. In order to determine whether this theory can indeed explain coronal heating, spectroscopic measurements are being compared to model nanoflare spectra. Such models have attempted to predict the spectra of impulsively heated plasmas in which the CSD is time dependent. These nonequilbirium ionization calculations have so far ignored EIMI, but our findings suggest that EIMI can have a significant effect on the CSD of a nanoflare-heated plasma, changing the ion abundances by up to about 50%.

  11. Charged-Particle Bean Transport for Ion Trapping Experiments.

    Science.gov (United States)

    Raichle, Brian W.; Wingfield, Love M.

    2001-11-01

    Electrostatic Einsel lenses are being developed for beam transport for use in two distinct metastable atomic lifetime experiments using two separate rf-ion traps. Each system has been modeled using Simion software, and the lenses have been designed from commercially available eV-parts. The first application is part of an electron gun source. Electrons are produced by a conventional dispenser cathode and are transported 25 cm to the trap. The design goal is to create a beam divergence to fully illuminate the active trap volume, and to provide tunable electron energies from 50 to 500 eV. The second application is to transport ions 1 m from a laser ablation ion source to an rf ion trap. Laser ablation involves essentially boiling ions from a solid target with intense laser pulses. Here, the design goal is to maximize flux by maximizing the solid angle of acceptance to the trap, minimize radial velocity, and minimize the spread in axial velocity. Development of a laser ablation ion source external to the trap volume will allow a very low base pressure in the trap region, which will make possible the study of species with lifetimes approaching 1 s. In addition, laser ablation will produce intermediately-charged ions from non-conductive solid targets.

  12. Telecloning Quantum States with Trapped Ions

    Institute of Scientific and Technical Information of China (English)

    2007-01-01

    We propose a scheme for telecloning quantum states with trapped ions. The scheme is based on a single ion interacting with a single laser pulse. In the protocol, an ion is firstly measured to determine whether the telecloning succeeds or not, and then another ion is detected to complete the whole procedure. The required experimental techniques are within the scope of what can be obtained in the ion-trap setup.

  13. Semiconductor characterization by scanning ion beam induced charge (IBIC) microscopy

    CERN Document Server

    Vittone, E; Olivero, P; Manfredotti, C; Jaksic, M; Giudice, A Lo; Fizzotti, F; Colombo, E

    2016-01-01

    The acronym IBIC (Ion Beam Induced Charge) was coined in early 1990's to indicate a scanning microscopy technique which uses MeV ion beams as probes to image the basic electronic properties of semiconductor materials and devices. Since then, IBIC has become a widespread analytical technique to characterize materials for electronics or for radiation detection, as testified by more than 200 papers published so far in peer-reviewed journals. Its success stems from the valuable information IBIC can provide on charge transport phenomena occurring in finished devices, not easily obtainable by other analytical techniques. However, IBIC analysis requires a robust theoretical background to correctly interpret experimental data. In order to illustrate the importance of using a rigorous mathematical formalism, we present in this paper a benchmark IBIC experiment aimed to test the validity of the interpretative model based on the Gunn's theorem and to provide an example of the analytical capability of IBIC to characteriz...

  14. Universal behavior of charged particle production in heavy ion collisions

    Science.gov (United States)

    Phobos Collaboration; Steinberg, Peter A.; Back, B. B.; Baker, M. D.; Barton, D. S.; Betts, R. R.; Ballintijn, M.; Bickley, A. A.; Bindel, R.; Budzanowski, A.; Busza, W.; Carroll, A.; Decowski, M. P.; Garcia, E.; George, N.; Gulbrandsen, K.; Gushue, S.; Halliwell, C.; Hamblen, J.; Heintzelman, G. A.; Henderson, C.; Hofman, D. J.; Hollis, R. S.; Hołński, R.; Holzman, B.; Iordanova, A.; Johnson, E.; Kane, J. L.; Katzy, J.; Khan, N.; Kucewicz, W.; Kulinich, P.; Kuo, C. M.; Lin, W. T.; Manly, S.; McLeod, D.; Michałowski, J.; Mignerey, A. C.; Nouicer, R.; Olszewski, A.; Pak, R.; Park, I. C.; Pernegger, H.; Reed, C.; Remsberg, L. P.; Reuter, M.; Roland, C.; Roland, G.; Rosenberg, L.; Sagerer, J.; Sarin, P.; Sawicki, P.; Skulski, W.; Steadman, S. G.; Steinberg, P.; Stephans, G. S. F.; Stodulski, M.; Sukhanov, A.; Tang, J.-L.; Teng, R.; Trzupek, A.; Vale, C.; van Nieuwenhuizen, G. J.; Verdier, R.; Wadsworth, B.; Wolfs, F. L. H.; Wosiek, B.; Woźniak, K.; Wuosmaa, A. H.; Wysłouch, B.

    2003-03-01

    The PHOBOS experiment at RHIC has measured the multiplicity of primary charged particles as a function of centrality and pseudorapidity in Au+Au collisions at sqrt(s_NN) = 19.6, 130 and 200 GeV. Two kinds of universal behavior are observed in charged particle production in heavy ion collisions. The first is that forward particle production, over a range of energies, follows a universal limiting curve with a non-trivial centrality dependence. The second arises from comparisons with pp/pbar-p and e+e- data. N_tot/(N_part/2) in nuclear collisions at high energy scales with sqrt(s) in a similar way as N_tot in e+e- collisions and has a very weak centrality dependence. This feature may be related to a reduction in the leading particle effect due to the multiple collisions suffered per participant in heavy ion collisions.

  15. Are There Topologically Charged States Associated with Quantum Electrodynamics ?

    CERN Document Server

    Marino, E C

    1994-01-01

    We present a formulation of Quantum Electrodynamics in terms of an antisymmetric tensor gauge field. In this formulation the topological current of this field appears as a source for the electromagnetic field and the topological charge therefore acts physically as an electric charge. The charged states of QED lie in the sector where the topological charge is identical to the matter charge. The antisymmetric field theory, however, admits new sectors where the topological charge is more general. These nontrivial, electrically charged, sectors contain massless states orthogonal to the vacuum which are created by a gauge invariant operator and can be interpreted as coherent states of photons. We evaluate the correlation functions of these states in the absence of matter. The new states have a positive definite norm and do interact with the charged states of QED in the usual way. It is argued that if these new sectors are in fact realized in nature then a very intense background electromagnetic field is necessary ...

  16. Electron emission and defect formation in the interaction of slow,highly charged ions with diamond surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Sideras-Haddad, E.; Shrivastava, S.; Rebuli, D.B.; Persaud, A.; Schneider, D.H.; Schenkel, T.

    2006-05-31

    We report on electron emission and defect formation in theinteraction between slow (v~;0.3 vBohr) highly charged ions (SHCI) withinsulating (type IIa) and semiconducting (type IIb) diamonds. Electronemission induced by 31Pq+ (q=5 to 13), and 136Xeq+ (q=34 to 44) withkinetic energies of 9 kVxq increase linearly with the ion charge states,reaching over 100 electrons per ion for high xenon charge states withoutsurface passivation of the diamond with hydrogen. Yields from bothdiamond types are up to a factor of two higher then from reference metalsurfaces. Crater like defects with diameters of 25 to 40 nm are formed bythe impact of single Xe44+ ions. High secondary electron yields andsingle ion induced defects enable the formation of single dopant arrayson diamond surfaces.

  17. X-ray And EUV Spectroscopy Of Highly Charged Tungsten Ions

    Science.gov (United States)

    Biedermann, Christoph; Radtke, Rainer

    2009-09-01

    The Berlin EBIT has been established by the Max-Planck-Institut für Plasmaphysik to generate atomic physics data in support of research in the field of controlled nuclear fusion, by measuring the radiation from highly charged ions in the x-ray, extreme ultraviolet and visible spectral ranges and providing valuable diagnostics for high temperature plasmas [1]. In future fusion devices, for example ITER, currently being constructed at Cadarache, France, the plasma facing components will be armored with high-Z materials, most likely tungsten, due to the favorable properties of this element [2]. At the same time the tremendous radiation cooling of these high-Z materials represents a threat to fusion and obliges one to monitor carefully the radiation. With EBIT a selected ensemble of ions in specific charge states can be produced, stored and excited for spectroscopic investigations. Employing this technique, we have for example resolved the wide structure observed around 5 nm at the ASDEX Upgrade tokamak as originating from E1-transitions into the open 4d shell of tungsten ions in charge states 25+ to 37+ producing a band-like emission pattern [3]. Further, these ions emit well-separated M1 lines in the EUV range around 65 nm suitable for plasma diagnostics [4]. Kr-like to Cr-like tungsten ions (38+ to 50+) show strong soft-x-ray lines in the range 0.5 to 2 and 5 to 15 nm. Lines of even higher charged tungsten ions, up to Ne-like W64+, abundant in the core plasma of present and future fusion test devices, have been investigated with high resolution Bragg-crystal spectroscopy at 0.13 nm [5]. Recently, x-ray spectroscopic measurements of the dielectronic recombination LMn resonances of W60+ to W67+ ions have been preformed and compare well with atomic structure calculations.

  18. Effects of Ions Charge-Mass Ratio on Energy and Energy Spread of Accelerated Ions in Laser Driven Plasma

    Institute of Scientific and Technical Information of China (English)

    SANG Hai-Bo; DENG Shi-Qiang; XIE Bai-Song

    2013-01-01

    Effects of ions charge-mass ratio on energy and energy spread of accelerated ions in laser driven plasma are investigated in detail by proposing a simple double-layer model for a foil target driven by an ultrastrong laser.The radiation pressure acceleration mechanism plays an important role on the studied problem.For the ions near the plasma mirror,i.e.electrons layer,the dependence of ions energy on their charge-mass ratio is derived theoretically.It is found that the larger the charge-mass ratio is,the higher the accelerated ions energy gets.For those ions far away from the layer,the dependence of energy and energy spread on ions charge-mass ratio are also obtained by numerical performance.It exhibits that,as ions charge-mass ratio increases,not only the accelerated ions energy but also the energy spread will become large.

  19. Counter-ions at Charged Walls: Two Dimensional Systems

    OpenAIRE

    Samaj, L.; Trizac, E.

    2010-01-01

    We study equilibrium statistical mechanics of classical point counter-ions, formulated on 2D Euclidean space with logarithmic Coulomb interactions (infinite number of particles) or on the cylinder surface (finite particle numbers), in the vicinity of a single uniformly charged line (one single double-layer), or between two such lines (interacting double-layers). The weak-coupling Poisson-Boltzmann theory, which applies when the coupling constant Gamma is small, is briefly recapitulated (the c...

  20. Two-photon processes in highly charged ions

    OpenAIRE

    Jahrsetz, Thorsten

    2015-01-01

    Two-photon processes are atomic processes in which an atom interacts simultaneously with two photons. Such processes describe a wide range of phenomena, such as two-photon decay and elastic or inelastic scattering of photons. In recent years two-photon processes involving highly charged heavy ions have become an active area of research. Such studies do not only consider the total transition or scattering rates but also their angular and polarization dependence. To support such examinations...