WorldWideScience

Sample records for bimolecular annihilation dynamics

  1. Analysis of Brownian Dynamics Simulations of Reversible Bimolecular Reactions

    KAUST Repository

    Lipková, Jana

    2011-01-01

    A class of Brownian dynamics algorithms for stochastic reaction-diffusion models which include reversible bimolecular reactions is presented and analyzed. The method is a generalization of the λ-bcȳ model for irreversible bimolecular reactions which was introduced in [R. Erban and S. J. Chapman, Phys. Biol., 6(2009), 046001]. The formulae relating the experimentally measurable quantities (reaction rate constants and diffusion constants) with the algorithm parameters are derived. The probability of geminate recombination is also investigated. © 2011 Society for Industrial and Applied Mathematics.

  2. RPMDrate: Bimolecular chemical reaction rates from ring polymer molecular dynamics

    KAUST Repository

    Suleimanov, Yu.V.

    2013-03-01

    We present RPMDrate, a computer program for the calculation of gas phase bimolecular reaction rate coefficients using the ring polymer molecular dynamics (RPMD) method. The RPMD rate coefficient is calculated using the Bennett-Chandler method as a product of a static (centroid density quantum transition state theory (QTST) rate) and a dynamic (ring polymer transmission coefficient) factor. The computational procedure is general and can be used to treat bimolecular polyatomic reactions of any complexity in their full dimensionality. The program has been tested for the H+H2, H+CH 4, OH+CH4 and H+C2H6 reactions. © 2012 Elsevier B.V. All rights reserved.

  3. Antinucleon-nucleon annihilation dynamics

    International Nuclear Information System (INIS)

    Myhrer, F.; Massachusetts Inst. of Tech., Cambridge

    1989-01-01

    The antinucleon-nucleon annihilation is predominantly described by a hot-fireball process where the many final quantum numbers are distributed in a statistical fashion. It is argued that caution must be used in employing the long-range meson-exchange forces to describe the protonium atomic states. The simplest processes of two final mesons do show puzzling behavior which might be a reflection of quark dynamics, but no guiding principles for these quark calculations have been established yet. (orig.)

  4. RPMDRATE: Bimolecular chemical reaction rates from ring polymer molecular dynamics

    Science.gov (United States)

    Suleimanov, Yu. V.; Allen, J. W.; Green, W. H.

    2013-03-01

    We present RPMDRATE, a computer program for the calculation of gas phase bimolecular reaction rate coefficients using the ring polymer molecular dynamics (RPMD) method. The RPMD rate coefficient is calculated using the Bennett-Chandler method as a product of a static (centroid density quantum transition state theory (QTST) rate) and a dynamic (ring polymer transmission coefficient) factor. The computational procedure is general and can be used to treat bimolecular polyatomic reactions of any complexity in their full dimensionality. The program has been tested for the H+H2, H+CH4, OH+CH4 and H+C2H6 reactions. Catalogue identifier: AENW_v1_0 Program summary URL: http://cpc.cs.qub.ac.uk/summaries/AENW_v1_0.html Program obtainable from: CPC Program Library, Queen's University, Belfast, N. Ireland Licensing provisions: MIT license No. of lines in distributed program, including test data, etc.: 94512 No. of bytes in distributed program, including test data, etc.: 1395674 Distribution format: tar.gz Programming language: Fortran 90/95, Python (version 2.6.x or later, including any version of Python 3, is recommended). Computer: Not computer specific. Operating system: Any for which Python, Fortran 90/95 compiler and the required external routines are available. Has the code been vectorized or parallelized?: The program can efficiently utilize 4096+ processors, depending on problem and available computer. At low temperatures, 110 processors are reasonable for a typical umbrella integration run with an analytic potential energy function and gradients on the latest x86-64 machines.

  5. Bimolecular reaction dynamics from photoelectron spectroscopy of negative ions

    International Nuclear Information System (INIS)

    Bradforth, S.E.

    1992-11-01

    The transition state region of a neutral bimolecular reaction may be experimentally investigated by photoelectron spectroscopy of an appropriate negative ion. The photoelectron spectrum provides information on the spectroscopy and dynamics of the short lived transition state and may be used to develop model potential energy surfaces that are semi-quantitative in this important region. The principles of bound → bound negative ion photoelectron spectroscopy are illustrated by way of an example: a full analysis of the photoelectron bands of CN - , NCO - and NCS - . Transition state photoelectron spectra are presented for the following systems Br + HI, Cl + HI, F + HI, F + CH 3 0H,F + C 2 H 5 OH,F + OH and F + H 2 . A time dependent framework for the simulation and interpretation of the bound → free transition state photoelectron spectra is subsequently developed and applied to the hydrogen transfer reactions Br + HI, F + OH → O( 3 P, 1 D) + HF and F + H 2 . The theoretical approach for the simulations is a fully quantum-mechanical wave packet propagation on a collinear model reaction potential surface. The connection between the wavepacket time evolution and the photoelectron spectrum is given by the time autocorrelation function. For the benchmark F + H 2 system, comparisons with three-dimensional quantum calculations are made

  6. Ab initio potential energy surfaces and quantum dynamics for polyatomic bimolecular reactions.

    Science.gov (United States)

    Fu, Bina; Zhang, Donghui

    2018-03-26

    There has been great progress in the development of potential energy surfaces (PESs) and quantum dynamics calculations in the gas phase. The establishment of fitting procedure for highly accurate PESs and new developments in quantum reactive scattering on reliable PESs allow accurate characterization of reaction dynamics beyond triatomic systems. This review will give the recent development in our group in constructing ab initio PESs based on the neural networks, and the time-dependent wave packet calculations for bimolecular reactions beyond three atoms. Bimolecular reactions of current interest to the community, namely, OH+H2, H+H2O, OH+CO, H+CH4 and Cl+CH4 are focused on. Quantum mechanical characterization of these reactions uncovers interesting dynamical phenomena with an unprecedented level of sophistication, and has greatly advanced our understanding of polyatomic reaction dynamics.

  7. The influence of the quencher concentration on the rate of simple bimolecular reaction: molecular dynamics study.

    Science.gov (United States)

    Litniewski, Marek

    2005-09-22

    The paper presents the results of large-scale molecular dynamics simulations of the irreversible bimolecular reaction A+B --> C+B for the simple liquid composed of mechanically identical soft spheres. The systems with the total number of molecules corresponding to 10(7)-10(9) are considered. The influence of the concentration of a quencher (B) on the surviving probability of A and the reaction rate is analyzed for a wide range of the concentrations and for two significantly different reduced densities. It is shown that the quencher concentration dependence effect (QCDE) is, in fact, a composition of two QCDE effects: the short-time QCDE that increases the reaction rate and the long-time QCDE that decreases it. The paper also analyzes the influence of the concentration on the steady-state rate constant, k(ss), obtained by integrating the surviving probability. The excess in k(ss) due to finite quencher concentration changes the sign from negative to positive while going from low to high concentrations. Generally, the excess is extremely weak. It attains a 1% level only if the concentration is very high.

  8. Exciton dynamics and annihilation in WS2 2D semiconductors.

    Science.gov (United States)

    Yuan, Long; Huang, Libai

    2015-04-28

    We systematically investigate the exciton dynamics in monolayered, bilayered, and trilayered WS2 two-dimensional (2D) crystals by time-resolved photoluminescence (TRPL) spectroscopy. The exciton lifetime when free of exciton annihilation was determined to be 806 ± 37 ps, 401 ± 25 ps, and 332 ± 19 ps for WS2 monolayer, bilayer, and trilayer, respectively. By measuring the fluorescence quantum yields, we also establish the radiative and nonradiative lifetimes of the direct and indirect excitons. The exciton decay in monolayered WS2 exhibits a strong excitation density-dependence, which can be described using an exciton-exciton annihilation (two-particle Auger recombination) model. The exciton-exciton annihilation rate for monolayered, bilayered, and trilayered WS2 was determined to be 0.41 ± 0.02, (6.00 ± 1.09) × 10(-3) and (1.88 ± 0.47) × 10(-3) cm(2) s(-1), respectively. Notably, the exciton-exciton annihilation rate is two orders of magnitude faster in the monolayer than in the bilayer and trilayer. We attribute the much slower exciton-exciton annihilation rate in the bilayer and trilayer to reduced many-body interaction and phonon-assisted exciton-exciton annihilation of indirect excitons.

  9. Molecular beam studies of unimolecular and bimolecular chemical reaction dynamics using VUV synchrotron radiation as a product probe

    Energy Technology Data Exchange (ETDEWEB)

    Blank, David Andrew [Univ. of California, Berkeley, CA (United States)

    1997-08-01

    This dissertation describes the use of a new molecular beam apparatus designed to use tunable VUV synchrotron radiation for photoionization of the products from scattering experiments. The apparatus was built at the recently constructed Advanced Light Source at Lawrence Berkeley National Laboratory, a third generation 1-2 GeV synchrotron radiation source. The new apparatus is applied to investigations of the dynamics of unimolecular reactions, photodissociation experiments, and bimolecular reactions, crossed molecular beam experiments. The first chapter describes the new apparatus and the VUV radiation used for photoionization. This is followed by a number of examples of the many advantages provided by using VUV photoionization in comparison with the traditional technique of electron bombardment ionization. At the end of the chapter there is a discussion of the data analysis employed in these scattering experiments. The remaining four chapters are complete investigations of the dynamics of four chemical systems using the new apparatus and provide numerous additional examples of the advantages provided by VUV photoionizaiton of the products. Chapters 2-4 are photofragment translational spectroscopy studies of the photodissociation dynamics of dimethyl sulfoxide, acrylonitrile, and vinyl chloride following absorption at 193 mn. All of these systems have multiple dissociation channels and provide good examples of the ability of the new apparatus to unravel the complex UV photodissociation dynamics that can arise in small polyatomic molecules.

  10. Role of vibrational dynamics in resonant positron annihilation on molecules.

    Science.gov (United States)

    Jones, A C L; Danielson, J R; Natisin, M R; Surko, C M

    2013-05-31

    Vibrational Feshbach resonances are dominant features of positron annihilation for incident positron energies in the range of the molecular vibrations. Studies in relatively small molecules are described that elucidate the role of intramolecular vibrational energy redistribution into near-resonant multimode states, and the subsequent coupling of these modes to the positron continuum, in suppressing or enhancing these resonances. The implications for annihilation in other molecular species, and the necessary ingredients of a more complete theory of resonant positron annihilation, are discussed.

  11. Dynamical effects of annihilation in pair-dominated winds

    Science.gov (United States)

    Becker, Peter A.; Begelman, Mitchell C.

    1990-01-01

    The steady, spherically symmetric flow of an ideal fluid dominated by photons and ultrarelativistic electron-positron pairs is analyzed. A new wind equation and a set of critical point conditions are obtained which describe the relativistic flow of an annihilation gas in which the flow velocity exceeds the diffusion velocity of the photons. Numerical results are reported which suggest the possible existence of trapped, pure-pair winds driven by the combined pressure of the pairs and the photons. Most of the annihilation occurs below the critical radius in trapped flows, and a substantial fraction of the total energy of the injected pairs is converted into kinetic energy and radiation. Accurate numerical solutions for the flow velocity and the positron loss rate in optically thin, Newtonian winds are obtained, and a useful approximate analytic relation between the positron loss rate and the flow velocity is derived which suggests that a large number of pairs may survive the annihilation region, ultimately escaping the potential well.

  12. Exciton Dynamics, Transport, and Annihilation in Atomically Thin Two-Dimensional Semiconductors.

    Science.gov (United States)

    Yuan, Long; Wang, Ti; Zhu, Tong; Zhou, Mingwei; Huang, Libai

    2017-07-20

    Large binding energy and unique exciton fine structure make the transition metal dichalcogenides (TMDCs) an ideal platform to study exciton behaviors in two-dimensional (2D) systems. While excitons in these systems have been extensively researched, there currently lacks a consensus on mechanisms that control dynamics. In this Perspective, we discuss extrinsic and intrinsic factors in exciton dynamics, transport, and annihilation in 2D TMDCs. Intrinsically, dark and bright exciton energy splitting is likely to play a key role in modulating the dynamics. Extrinsically, defect scattering is prevalent in single-layer TMDCs, which leads to rapid picosecond decay and limits exciton transport. The exciton-exciton annihilation process in single-layer TMDCs is highly efficient, playing an important role in the nonradiative recombination rate in the high exciton density regime. Future challenges and opportunities to control exciton dynamics are discussed.

  13. Annihilating vacancies via dynamic reflection and emission of interstitials in nano-crystal tungsten

    Science.gov (United States)

    Li, Xiangyan; Duan, Guohua; Xu, Yichun; Zhang, Yange; Liu, Wei; Liu, C. S.; Liang, Yunfeng; Chen, Jun-Ling; Luo, G.-N.

    2017-11-01

    Radiation damage not only seriously degrades the mechanical properties of tungsten (W) but also enhances hydrogen retention in the material. Introducing a large amount of defect sinks, e.g. grain boundaries (GBs) is an effective method for improving radiation-resistance of W. However, the mechanism by which the vacancies are dynamically annihilated at long timescale in nano-crystal W is still not clear. The dynamic picture for eliminating vacancies with single interstitials and small interstitial-clusters has been investigated by combining molecular dynamics, molecular statics and object Kinetic Monte Carlo methods. On one hand, the annihilation of bulk vacancies was enhanced due to the reflection of an interstitial-cluster of parallel ≤ftright> crowdions by the GB. The interstitial-cluster was observed to be reflected back into the grain interior when approaching a locally dense GB region. Near this region, the energy landscape for the interstitial was featured by a shoulder, different to the decreasing energy landscape of the interstitial near a locally loose region as indicative of the sink role of the GB. The bulk vacancy on the reflection path was annihilated. On the other hand, the dynamic interstitial emission efficiently anneals bulk vacancies. The single interstitial trapped at the GB firstly moved along the GB quickly and clustered to be the di-interstitial therein, reducing its mobility to a value comparable to that that for bulk vacancy diffusion. Then, the bulk vacancy was recombined via the coupled motion of the di-interstitial along the GB, the diffusion of the vacancy towards the GB and the accompanying interstitial emission. These results suggest that GBs play an efficient role in improving radiation-tolerance of nano-crystal W via reflecting highly-mobile interstitials and interstitial-clusters into the bulk and annihilating bulk vacancies, and via complex coupling of in-boundary interstitial diffusion, clustering of the interstitial and vacancy

  14. Separating annihilation and excitation energy transfer dynamics in light harvesting systems.

    Science.gov (United States)

    Vengris, Mikas; Larsen, Delmar S; Valkunas, Leonas; Kodis, Gerdenis; Herrero, Christian; Gust, Devens; Moore, Thomas; Moore, Ana; van Grondelle, Rienk

    2013-09-26

    The dependence of excitation energy transfer kinetics on the electronic state of the acceptor (ground vs excited) has been resolved with a novel multipulse prePump-Pump-Probe spectroscopy. The primary energy transfer and annihilation dynamics in two model light-harvesting systems were explored: an artificially synthesized carotenoid-zinc-phthalocyanine dyad and a naturally occurring light-harvesting peridinin-chlorophyll protein complex from Amphidinium carterae. Both systems use carotenoid as the primary excitation energy donor with porphyrin chromophores as the acceptor molecules. The prePump-Pump-Probe transient signals were analyzed with Monte Carlo modeling to explicitly address the underlying step-by-step kinetics involved in both excitation migration and annihilation processes. Both energy transfer and annihilation dynamics were demonstrated to occur with approximately the same rate in both systems, regardless of the excitation status of the acceptor pigments. The possible reasons for these observations are discussed in the framework of the Förster energy transfer model.

  15. Dynamics and heat diffusion of Abrikosov's vortex-antivortex pairs during an annihilation process.

    Science.gov (United States)

    Duarte, E C S; Sardella, E; Ortiz, W A; Zadorosny, R

    2017-10-11

    The manipulation and control of vortex states in superconducting systems are of great interest in view of possible applications, for which mesoscopic materials are good candidates. In this work, we studied the annihilation dynamics and the dissipative aspects of an Abrikosov's vortex-antivortex pair in a mesoscopic superconducting system with a concentric hole. The generalized time-dependent Ginzburg-Landau equations were numerically solved. The main result is the appearance of a phase slip-like line due to the elongation of the vortex and antivortex cores. Under specific circumstances, thermal dissipation might be associated with a sizeable relaxation of the order parameter, so that the energy released in the annihilation of a vortex-antivortex pair might become detectable in measurements of the magnetization as a function of time.

  16. Dynamics of vortex-antivortex creation and annihilation in current-driven mesoscopic superconducting squares

    Science.gov (United States)

    Liang, Xiao-Meng; Zha, Guo-Qiao

    2015-12-01

    In this paper, based on the time-dependent Ginzburg-Landau theory, we study the dynamics of vortex-antivortex (V-Av) pairs in a mesoscopic superconducting square with a small hole under applied bias currents. For the sample with a centered hole, a V-Av pair can nucleate at the hole edges and moves in opposite directions perpendicular to applied constant DC drive. The influence of the external magnetic field on the (anti)vortex velocity and the lifetime of V-Av pairs is mainly investigated. Different modes in the dynamical process of the V-Av collision and annihilation are identified. Moreover, in the case when the hole is displaced from the center of the square, the V-Av dynamics behaves quite differently from the symmetric case due to the shift of the V-Av creation point.

  17. Vacancy profile in reverse osmosis membranes studied by positron annihilation lifetime measurements and molecular dynamics simulations

    International Nuclear Information System (INIS)

    Shimazu, A; Shintani, T; Hirose, M; Goto, H; Suzuki, R; Kobayashi, Y

    2013-01-01

    The positron annihilation technique using a slow positron beam can be used for the study of the vacancy profiles in typical reverse osmosis (RO) membranes. In this study, the vacancy profile in the polyamide membrane that exhibits a high permselectivity between ions and water was studied using the positron annihilation technique and molecular dynamics simulations. Ortho-positronium (o-Ps) lifetimes in the surface region of the membranes were evaluated by using a slow positron beam. The diffusion behavior of Na + and water in the polyamides was simulated by molecular dynamics (MD) methods using the TSUBAME2 supercomputer at the Tokyo Institute of Technology and discussed with the vacancy profile probed by the o-Ps. The results suggested that the large hydration size of Na + compared to the vacancy size in the polyamides contributes to the increased diffusivity selectivity of water/Na + that is related to the NaCl desalination performance of the membrane. Both the hydration size of the ions and the vacancy size appeared to be significant parameters to discuss the diffusivity selectivity of water/ions in typical polyamide membranes.

  18. Charge recombination and exciton annihilation reactions in conjugated polymer blends.

    Science.gov (United States)

    Howard, Ian A; Hodgkiss, Justin M; Zhang, Xinping; Kirov, Kiril R; Bronstein, Hugo A; Williams, Charlotte K; Friend, Richard H; Westenhoff, Sebastian; Greenham, Neil C

    2010-01-13

    Bimolecular interactions between excitations in conjugated polymer thin films are important because they influence the efficiency of many optoelectronic devices that require high excitation densities. Using time-resolved optical spectroscopy, we measure the bimolecular interactions of charges, singlet excitons, and triplet excitons in intimately mixed polyfluorene blends with band-edge offsets optimized for photoinduced electron transfer. Bimolecular charge recombination and triplet-triplet annihilation are negligible, but exciton-charge interactions are efficient. The annihilation of singlet excitons by charges occurs on picosecond time-scales and reaches a rate equivalent to that of charge transfer. Triplet exciton annihilation by charges occurs on nanosecond time-scales. The surprising absence of nongeminate charge recombination is shown to be due to the limited mobility of charge carriers at the heterojunction. Therefore, extremely high densities of charge pairs can be maintained in the blend. The absence of triplet-triplet annihilation is a consequence of restricted triplet diffusion in the blend morphology. We suggest that the rate and nature of bimolecular interactions are determined by the stochastic excitation distribution in the polymer blend and the limited connectivity between the polymer domains. A model based on these assumptions quantitatively explains the effects. Our findings provide a comprehensive framework for understanding bimolecular recombination and annihilation processes in nanostructured materials.

  19. Selection rules for bimolecular photoabsorption

    Science.gov (United States)

    Andrews, David L.; Bittner, Alexander M.

    1992-09-01

    Bimolecular photoabsorption is a term describing processes in which two molecules or other chemically distinct entities undergo simultaneous excitation to electronic excited states, the energy being provided by the absorption of one or more laser photons. These processes have previously been referred to as synergistic, cooperative, or mean-frequency absorption. This paper introduces a new terminology for the description of such phenomena and provides an overview of the features associated with bimolecular processes involving the absorption of one, two or three photons from a single laser beam. Emphasis is placed on a detailed symmetry analysis based on irreducible tensors, leading to a comprehensive treatment of the selection rules for all the major molecular point groups. Finally, attention is drawn to some systems in which these effects have been detected, and others in which they might be expected to occur.

  20. Bimolecular reactions of carbenes: Proton transfer mechanism

    Science.gov (United States)

    Abu-Saleh, Abd Al-Aziz A.; Almatarneh, Mansour H.; Poirier, Raymond A.

    2018-04-01

    Here we report the bimolecular reaction of trifluoromethylhydroxycarbene conformers and the water-mediated mechanism of the 1,2-proton shift for the unimolecular trans-conformer by using quantum chemical calculations. The CCSD(T)/cc-pVTZ//MP2/cc-pVDZ potential-energy profile of the bimolecular reaction of cis- and trans-trifluoromethylhydroxycarbene, shows the lowest gas-phase barrier height of 13 kJ mol-1 compared to the recently reported value of 128 kJ mol-1 for the unimolecular reaction. We expect bimolecular reactions of carbene's stereoisomers will open a valuable field for new and useful synthetic strategies.

  1. Free volume study on the miscibility of PEEK/PEI blend using positron annihilation and dynamic mechanical thermal analysis

    International Nuclear Information System (INIS)

    Ramani, R; Alam, S

    2015-01-01

    High performance polymer blend of poly(ether ether ketone) (PEEK) and poly(ether imide) (PEI) was examined for their free volume behaviour using positron annihilation lifetime spectroscopy and dynamic mechanical thermal analysis methods. The fractional free volume obtained from PALS shows a negative deviation from linear additivity rule implying good miscibility between PEEK and PEI. The dynamic modulus and loss tangent were obtained for the blends at three different frequencies 1, 10 and 100 Hz at temperatures close to and above their glass transition temperature. Applying Time-Temperature-Superposition (TTS) principle to the DMTA results, master curves were obtained at a reference temperature T o and the WLF coefficients c 0 1 and c 0 2 were evaluated. Both the methods give similar results for the dependence of fractional free volume on PEI content in this blend. The results reveal that free volume plays an important role in determining the visco-elastic properties in miscible polymer blends. (paper)

  2. Flavoured co-annihilation

    Indian Academy of Sciences (India)

    2012-10-06

    annihilating part- ners of the neutralino is the lightest stau, ˜τ1. In the presence of flavour violation in the right-handed sector, the co-annihilating partner would be a flavour mixed state. The flavour effect is two-fold: (a) It changes the ...

  3. On the Role of the Annihilation Channel in Front Form Positronium

    OpenAIRE

    Trittmann, Uwe

    1997-01-01

    The annihilation channel is implemented into the front form calculations of the positronium spectrum presented in a previous publication. The effective Hamiltonian is calculated analytically. Its eigensolutions are obtained numerically. A complete separation of the dynamical and instantaneous part of the annihilation interaction is observed. We find the remarkable effect that the annihilation channel stabilizes the cutoff behavior of the spectrum.

  4. Perspective: Vibrational-induced steric effects in bimolecular reactions

    Energy Technology Data Exchange (ETDEWEB)

    Liu, Kopin, E-mail: kliu@po.iams.sinica.edu.tw [Institute of Atomic and Molecular Sciences (IAMS), Academia Sinica, P.O. Box 23-166, Taipei 10617, Taiwan (China)

    2015-02-28

    The concept of preferred collision geometry in a bimolecular reaction is at the heart of reaction dynamics. Exemplified by a series of crossed molecular beam studies on the reactions of a C–H stretch-excited CHD{sub 3}(v{sub 1} = 1) with F, Cl, and O({sup 3}P) atoms, two types of steric control of chemical reactivity will be highlighted. A passive control is governed in a reaction with strong anisotropic entry valley that can significantly steer the incoming trajectories. This disorientation effect is illustrated by the F and O({sup 3}P) + CHD{sub 3}(v{sub 1} = 1) reactions. In the former case, the long-range anisotropic interaction acts like an optical “negative” lens by deflecting the trajectories away from the favored transition-state geometry, and thus inhibiting the bond rupture of the stretch-excited CHD{sub 3}. On the contrary, the interaction between O({sup 3}P) and CHD{sub 3}(v{sub 1} = 1) behaves as a “positive” lens by funneling the large impact-parameter collisions into the cone of acceptance, and thereby enhances the reactivity. As for reactions with relatively weak anisotropic interactions in the entry valley, an active control can be performed by exploiting the polarization property of the infrared excitation laser to polarize the reactants in space, as demonstrated in the reaction of Cl with a pre-aligned CHD{sub 3}(v{sub 1} = 1) reactant. A simpler case, the end-on versus side-on collisions, will be elucidated for demonstrating a means to disentangle the impact-parameter averaging. A few general remarks about some closely related issues, such as mode-, bond-selectivity, and Polanyi’s rules, are made.

  5. Construction of a bimolecular fluorescence complementation (BiFC ...

    African Journals Online (AJOL)

    Protein–protein interactions are essential for signal transduction in cells. Bimolecular fluorescence complementation (BiFC) is a novel technology that utilises green fluorescent proteins to visualize protein–protein interactions and subcellular protein localisation. BiFC based on pSATN vectors are a good system for ...

  6. Diabolo creation and annihilation.

    Science.gov (United States)

    Freund, Isaac; Soskin, Marat S; Egorov, Roman I; Denisenko, Vladimir

    2006-08-15

    A point of circular polarization embedded in a paraxial field of elliptical polarization is a polarization singularity called a C point. At such a point the major axis a and minor axis b of the ellipse become degenerate. Away from the C point this degeneracy is lifted such that surfaces a and b form nonanalytic cones that are joined at their apex (the C point) to produce a double cone called a diabolo. Typically, during propagation diabolo pairs are created or annihilated. We present rules based on geometry and topology that govern these events, provide initial experimental confirmation, and enumerate the allowed configurations in which diabolos can be created or annihilated.

  7. Positron annihilation microprobe

    Energy Technology Data Exchange (ETDEWEB)

    Canter, K.F. [Brandeis Univ., Waltham, MA (United States)

    1997-03-01

    Advances in positron annihilation microprobe development are reviewed. The present resolution achievable is 3 {mu}m. The ultimate resolution is expected to be 0.1 {mu}m which will enable the positron microprobe to be a valuable tool in the development of 0.1 {mu}m scale electronic devices in the future. (author)

  8. Positron annihilation processes update

    Science.gov (United States)

    Guessoum, Nidhal; Skibo, Jeffrey G.; Ramaty, Reuven

    1997-01-01

    The present knowledge concerning the positron annihilation processes is reviewed, with emphasis on the data of the cross sections of the various processes of interest in astrophysical applications. Recent results are presented including results on reaction rates and line widths, the validity of which is verified.

  9. Understanding bimolecular machines: Theoretical and experimental approaches

    Science.gov (United States)

    Goler, Adam Scott

    This dissertation concerns the study of two classes of molecular machines from a physical perspective: enzymes and membrane proteins. Though the functions of these classes of proteins are different, they each represent important test-beds from which new understanding can be developed by the application of different techniques. HIV1 Reverse Transcriptase is an enzyme that performs multiple functions, including reverse transcription of RNA into an RNA/DNA duplex, RNA degradation by the RNaseH domain, and synthesis of dsDNA. These functions allow for the incorporation of the retroviral genes into the host genome. Its catalytic cycle requires repeated large-scale conformational changes fundamental to its mechanism. Motivated by experimental work, these motions were studied theoretically by the application of normal mode analysis. It was observed that the lowest order modes correlate with largest amplitude (low-frequency) motion, which are most likely to be catalytically relevant. Comparisons between normal modes obtained via an elastic network model to those calculated from the essential dynamics of a series of all-atom molecular dynamics simulations show the self-consistency between these calculations. That similar conformational motions are seen between independent theoretical methods reinforces the importance of large-scale subdomain motion for the biochemical action of DNA polymerases in general. Moreover, it was observed that the major subunits of HIV1 Reverse Transcriptase interact quasi-harmonically. The 5HT3A Serotonin receptor and P2X1 receptor, by contrast, are trans-membrane proteins that function as ligand gated ion channels. Such proteins feature a central pore, which allows for the transit of ions necessary for cellular function across a membrane. The pore is opened by the ligation of binding sites on the extracellular portion of different protein subunits. In an attempt to resolve the individual subunits of these membrane proteins beyond the diffraction

  10. Bubble chamber: antiproton annihilation

    CERN Multimedia

    1971-01-01

    These images show real particle tracks from the annihilation of an antiproton in the 80 cm Saclay liquid hydrogen bubble chamber. A negative kaon and a neutral kaon are produced in this process, as well as a positive pion. The invention of bubble chambers in 1952 revolutionized the field of particle physics, allowing real tracks left by particles to be seen and photographed by expanding liquid that had been heated to boiling point.

  11. Theory of Crowding Effects on Bimolecular Reaction Rates.

    Science.gov (United States)

    Berezhkovskii, Alexander M; Szabo, Attila

    2016-07-07

    An analytical expression for the rate constant of a diffusion-influenced bimolecular reaction in a crowded environment is derived in the framework of a microscopic model that accounts for: (1) the slowdown of diffusion due to crowding and the dependence of the diffusivity on the distance between the reactants, (2) a crowding-induced attractive short-range potential of mean force, and (3) nonspecific reversible binding to the crowders. This expression spans the range from reaction to diffusion control. Crowding can increase the reaction-controlled rate by inducing an effective attraction between reactants but decrease the diffusion-controlled rate by reducing their relative diffusivity.

  12. Experimental Determination of Gas Phase Thermodynamic Properties of Bimolecular Complexes

    Science.gov (United States)

    Hansen, Anne S.; Maroun, Zeina; Mackeprang, Kasper; Kjaergaard, Henrik G.

    2016-06-01

    Accurate determination of the atmospheric abundance of hydrogen bound bimolecular complexes is necessary, as hydrogen bonds are partly responsible for the formation and growth of aerosol particles. The abundance of a complex is related to the Gibbs free energy of complex formation (Δ G), which is often obtained from quantum chemical calculations that rely on calculated values of the enthalpy (Δ H) and entropy (Δ S) of complex formation. However, calculations of Δ H and in particular Δ S are associated with large uncertainties, and accurate experimental values are therefore crucial for theoretical benchmarking studies. Infrared measurements of gas phase hydrogen bound complexes were performed in the 300 to 373 K range, and lead to a purely experimental determination of Δ H using the van't Hoff equation. Equilibrium constants were determined by combining an experimental and calculated OH-stretching intensity, from which values of Δ G and hence Δ S could be determined. Thus we can determine Δ G, Δ H and Δ S for a bimolecular complex. We find that in the 300 to 373 K temperature range the determined Δ H and Δ S values are independent of temperature.

  13. Biological Effectiveness of Antiproton Annihilation

    DEFF Research Database (Denmark)

    Maggiore, C.; Agazaryan, N.; Bassler, N.

    2004-01-01

    from the annihilation of antiprotons produce an increase in ‘‘biological dose’’ in the vicinity of the narrow Bragg peak for antiprotons compared to protons. This experiment is the first direct measurement of the biological effects of antiproton annihilation. The background, description, and status...

  14. Positron scattering and annihilation from hydrogenlike ions

    International Nuclear Information System (INIS)

    Novikov, S.A.; Bromley, M.W.J.; Mitroy, J.

    2004-01-01

    The Kohn variational method is used with a configuration-interaction-type wave function to determine the J=0 and J=1 phase shifts and annihilation parameter Z eff for positron-hydrogenic ion scattering. The phase shifts are within 1-2% of the best previous calculations. The values of Z eff are small and do not exceed unity for any of the momenta considered. At thermal energies Z eff is minute with a value of order 10 -50 occurring for He + at k=0.05a 0 -1 . In addition to the variational calculations, analytic expressions for the phase shift and annihilation parameters within the Coulomb wave Born approximation are derived and used to help elucidate the dynamics of positron collisions with positive ions

  15. Controlling Positronium Annihilation with Electric Fields.

    Science.gov (United States)

    Alonso, A M; Cooper, B S; Deller, A; Hogan, S D; Cassidy, D B

    2015-10-30

    We show that the annihilation dynamics of excited positronium (Ps) atoms can be controlled using parallel electric and magnetic fields. To achieve this, Ps atoms were optically excited to n=2 sublevels in fields that were adjusted to control the amount of short-lived and long-lived character of the resulting mixed states. Inclusion of the former offers a practical approach to detection via annihilation radiation, whereas the increased lifetimes due to the latter can be exploited to optimize resonance-enhanced two-photon excitation processes (e.g., 1^{3}S→2^{3}P→nS/nD), either by minimizing losses through intermediate state decay, or by making it possible to separate the excitation laser pulses in time. In addition, photoexcitation of mixed states with a 2^{3}S_{1} component represents an efficient route to producing long-lived pure 2^{3}S_{1} atoms via single-photon excitation.

  16. Kinetics and mechanism of bimolecular electron transfer reaction in quinone-amine systems in micellar solution

    International Nuclear Information System (INIS)

    Kumbhakar, Manoj; Nath, Sukhendu; Mukherjee, Tulsi; Pal, Haridas

    2005-01-01

    Photoinduced electron transfer (ET) reactions between anthraquinone derivatives and aromatic amines have been investigated in sodium dodecyl sulphate (SDS) micellar solutions. Significant static quenching of the quinone fluorescence due to high amine concentration in the micellar phase has been observed in steady-state measurements. The bimolecular rate constants for the dynamic quenching in the present systems k q TR , as estimated from the time-resolved measurements, have been correlated with the free energy changes ΔG 0 for the ET reactions. Interestingly it is seen that the k q TR vs ΔG 0 plot displays an inversion behavior with maximum k q TR at around 0.7 eV, a trend similar to that predicted in Marcus ET theory. Like the present results, Marcus inversion in the k q TR values was also observed earlier in coumarin-amine systems in SDS and TX-100 micellar solutions, with maximum k q TR at around the same exergonicity. These results thus suggest that Marcus inversion in bimolecular ET reaction is a general phenomenon in micellar media. Present observations have been rationalized on the basis of the two-dimensional ET (2DET) theory, which seems to be more suitable for micellar ET reactions than the conventional ET theory. For the quinone-amine systems, it is interestingly seen that k q TR vs ΔG 0 plot is somewhat wider in comparison to that of the coumarin-amine systems, even though the maxima in the k q TR vs ΔG 0 plots appear at almost similar exergonicity for both the acceptor-donor systems. These observations have been rationalized on the basis of the differences in the reaction windows along the solvation axis, as envisaged within the framework of the 2DET theory, and arise due to the differences in the locations of the quinones and coumarin dyes in the micellar phase

  17. Correlated Pair States Formed by Singlet Fission and Exciton-Exciton Annihilation.

    Science.gov (United States)

    Scholes, Gregory D

    2015-12-24

    Singlet fission to form a pair of triplet excitations on two neighboring molecules and the reverse process, triplet-triplet annihilation to upconvert excitation, have been extensively studied. Comparatively little work has sought to examine the properties of the intermediate state in both of these processes-the bimolecular pair state. Here, the eigenstates constituting the manifold of 16 bimolecular pair excitations and their relative energies in the weak-coupling regime are reported. The lowest-energy states obtained from the branching diagram method are the triplet pairs with overall singlet spin |X1⟩ ≈ (1)[TT] and quintet spin |Q⟩ ≈ (5)[TT]. It is shown that triplet pair states can be separated by a triplet-triplet energy-transfer mechanism to give a separated, yet entangled triplet pair (1)[T···T]. Independent triplets are produced by decoherence of the separated triplet pair. Recombination of independent triplets by exciton-exciton annihilation to form the correlated triplet pair (i.e., nongeminate recombination) happens with 1/3 of the rate of either triplet migration or recombination of the separated correlated triplet pair (geminate recombination).

  18. Brane annihilations during inflation

    International Nuclear Information System (INIS)

    Battefeld, Diana; Battefeld, Thorsten; Firouzjahi, Hassan; Khosravi, Nima

    2010-01-01

    We investigate brane inflation driven by two stacks of mobile branes in a throat. The stack closest to the bottom of the throat annihilates first with antibranes, resulting in particle production and a change of the equation of state parameter w. We calculate analytically some observable signatures of the collision; related decays are common in multi-field inflation, providing the motivation for this case study. The discontinuity in w enters the matching conditions relating perturbations in the remaining degree of freedom before and after the collision, affecting the power-spectrum of curvature perturbations. We find an oscillatory modulation of the power-spectrum for scales within the horizon at the time of the collision, and a slightly redder spectrum on super-horizon scales. We comment on implications for staggered inflation

  19. Diffuse galactic annihilation radiation

    Science.gov (United States)

    Ramaty, R.; Lingenfelter, R. E.

    1993-01-01

    The study reports observations of positron annihilation radiation from the inner region of the Galaxy which show that there are two components of the radiation: a steady, diffuse Galactic component and a variable component from discrete, presumably compact sources. The existence of the variable component is supported by the ensemble of all narrow FOV 511 keV line observations, including recent detections with OSSE. The fit of this ensemble to a time-independent source distribution can be excluded at the approximately 3-sigma level. The same ensemble, combined with the broad FOV SMM observations of Galactic 511 keV line emission, sets constraints on the Galactic distribution of the diffuse component.

  20. Positron annihilation in superconductive metals

    Energy Technology Data Exchange (ETDEWEB)

    Dekhtjar, I.J.

    1969-03-10

    A correlation is shown between the parameters of superconductive metals and those of positron annihilation. Particular attention is paid to the density states obtained from the electron specific heat.

  1. Annihilation in Gases and Galaxies

    Science.gov (United States)

    Drachman, Richard J. (Editor)

    1990-01-01

    This publication contains most of the papers, both invited and contributed, that were presented at the Workshop of Annihilation in Gases and Galaxies. This was the fifth in a biennial series associated with the International Conference on the Physics of Electronic and Atomic Collisions. Subjects covered included the scattering and annihilation of positrons and positronium atoms in various media, including those of astrophysical interest. In addition, the topics of antimatter and dark matter were covered.

  2. ATHENA: an actual antihydrogen annihilation

    CERN Document Server

    2002-01-01

    This is an image of an actual matter-antimatter annihilation due to an atom of antihydrogen in the ATHENA experiment, located on the Antiproton Decelerator (AD) at CERN since 2001. The antiproton produces four charged pions (yellow) whose positions are given by silicon microstrips (pink) before depositing energy in CsI crystals (yellow cubes). The positron also annihilates to produce back-to-back gamma rays (red).

  3. Bimolecular Recombination Kinetics of an Exciton-Trion Gas

    Science.gov (United States)

    2015-07-01

    particles are created and annihilated in pairs so that there is no accumulation of charge. However, this approach is rigorously correct only for a...8 ~ ( )22 23.75 10 photons/ cm s× ⋅ . A quantum yield for electron-hole pair creation of 0.004 would create a generation flux G within the...hole pairs , magenta—excitons, and blue—trions. The final parameter of interest is Q, which controls the creation of excitons by electron–hole

  4. Very Low Rate Constants of Bimolecular CO Adsorption on Anionic Gold Clusters: Implications for Catalytic Activity

    Czech Academy of Sciences Publication Activity Database

    Balteanu, I.; Balaj, O. P.; Fox, B. S.; Beyer, M. K.; Bastl, Zdeněk; Bondybey, V. E.

    2003-01-01

    Roč. 5, - (2003), s. 1213-1218 ISSN 1463-9076 Institutional research plan: CEZ:AV0Z4040901 Keywords : bimolecular * adsorption * catalytic activity Subject RIV: CF - Physical ; Theoretical Chemistry Impact factor: 1.959, year: 2003

  5. Two-exciton excited states of J-aggregates in the presence of exciton–exciton annihilation

    International Nuclear Information System (INIS)

    Levinsky, B.; Fainberg, B.D.; Nesterov, L.A.; Rosanov, N.N.

    2016-01-01

    We study decay of two-exciton states of a J-aggregate that is collective in nature. We use mathematical formalism based on effective non-Hermitian Hamiltonian suggested in nuclear theory. We show that decay of two-exciton states is strongly affected by the interference processes in the exciton–exciton annihilation. Our evaluations of the imaginary part of the effective Hamiltonian show that it exceeds the spacing between real energies of the two-exciton states that gives rise to the transition to the regime of overlapping resonances supplying the system by the new collectivity – the possibility of coherent decay in the annihilation channel. The decay of two-exciton states varies from twice bimolecular decay rate to the much smaller values that is associated with population trapping. We have also considered the corresponding experiment in the framework of our approach, the picture of which appears to be more complex and richer than it was reasoned before.

  6. Biological effectiveness of antiproton annihilation

    CERN Document Server

    Holzscheiter, Michael H.; Bassler, Niels; Beyer, Gerd; De Marco, John J.; Doser, Michael; Ichioka, Toshiyasu; Iwamoto, Keisuke S.; Knudsen, Helge V.; Landua, Rolf; Maggiore, Carl; McBride, William H.; Møller, Søren Pape; Petersen, Jorgen; Smathers, James B.; Skarsgard, Lloyd D.; Solberg, Timothy D.; Uggerhøj, Ulrik I.; Withers, H.Rodney; Vranjes, Sanja; Wong, Michelle; Wouters, Bradly G.

    2004-01-01

    We describe an experiment designed to determine whether or not the densely ionizing particles emanating from the annihilation of antiprotons produce an increase in “biological dose” in the vicinity of the narrow Bragg peak for antiprotons compared to protons. This experiment is the first direct measurement of the biological effects of antiproton annihilation. The experiment has been approved by the CERN Research Board for running at the CERN Antiproton Decelerator (AD) as AD-4/ACE (Antiproton Cell Experiment) and has begun data taking in June of 2003. The background, description and the current status of the experiment are given.

  7. Biological effectiveness of antiproton annihilation

    DEFF Research Database (Denmark)

    Holzscheiter, M.H.; Agazaryan, N.; Bassler, Niels

    2004-01-01

    We describe an experiment designed to determine whether or not the densely ionizing particles emanating from the annihilation of antiprotons produce an increase in ‘‘biological dose’’ in the vicinity of the narrow Bragg peak for antiprotons compared to protons. This experiment is the first direct...... measurement of the biological effects of antiproton annihilation. The experiment has been approved by the CERN Research Board for running at the CERN Antiproton Decelerator (AD) as AD-4/ACE (Antiproton Cell Experiment) and has begun data taking in June of 2003. The background, description and the current...

  8. Positron annihilation near fractal surfaces

    International Nuclear Information System (INIS)

    Lung, C.W.; Deng, K.M.; Xiong, L.Y.

    1991-07-01

    A model for positron annihilation in the sub-surface region near a fractal surface is proposed. It is found that the power law relationship between the mean positron implantation depth and incident positron energy can be used to measure the fractal dimension of the fractal surface in materials. (author). 10 refs, 2 figs

  9. Selection Rule for Enhanced Dark Matter Annihilation.

    Science.gov (United States)

    Das, Anirban; Dasgupta, Basudeb

    2017-06-23

    We point out a selection rule for enhancement (suppression) of odd (even) partial waves of dark matter coannihilation or annihilation using the Sommerfeld effect. Using this, the usually velocity-suppressed p-wave annihilation can dominate the annihilation signals in the present Universe. The selection mechanism is a manifestation of the exchange symmetry of identical incoming particles, and generic for multistate DM with off-diagonal long-range interactions. As a consequence, the relic and late-time annihilation rates are parametrically different and a distinctive phenomenology, with large but strongly velocity-dependent annihilation rates, is predicted.

  10. Photoinduced bimolecular electron transfer kinetics in small unilamellar vesicles

    International Nuclear Information System (INIS)

    Choudhury, Sharmistha Dutta; Kumbhakar, Manoj; Nath, Sukhendu; Pal, Haridas

    2007-01-01

    Photoinduced electron transfer (ET) from N,N-dimethylaniline to some coumarin derivatives has been studied in small unilamellar vesicles (SUVs) of the phospholipid, DL-α-dimyristoyl-phosphatidylcholine, using steady-state and time-resolved fluorescence quenching, both below and above the phase transition temperature of the vesicles. The primary interest was to examine whether Marcus inversion [H. Sumi and R. A. Marcus, J. Chem. Phys. 84, 4894 (1986)] could be observed for the present ET systems in these organized assemblies. The influence of the topology of SUVs on the photophysical properties of the reactants and consequently on their ET kinetics has also been investigated. Absorption and fluorescence spectral data of the coumarins in SUVs and the variation of their fluorescence decays with temperature indicate that the dyes are localized in the bilayer of the SUVs. Time-resolved area normalized emission spectra analysis, however, reveals that the dyes are distributed in two different microenvironments in the SUVs, which we attribute to the two leaflets of the bilayer, one toward bulk water and the other toward the inner water pool. The microenvironments in the two leaflets are, however, not indicated to be that significantly different. Time-resolved anisotropy decays were biexponential for all the dyes in SUVs, and this has been interpreted in terms of the compound motion model according to which the dye molecules can experience a fast wobbling-in-cone type of motion as well as a slow overall rotating motion of the cone containing the molecule. The expected bimolecular diffusion-controlled rates in SUVs, as estimated by comparing the microviscosities in SUVs (determined from rotational correlation times) and that in acetonitrile solution, are much slower than the observed fluorescence quenching rates, suggesting that reactant diffusion (translational) does not play any role in the quenching kinetics in the present systems. Accordingly, clear inversions are

  11. Multiple gamma lines from semi-annihilation

    International Nuclear Information System (INIS)

    D'Eramo, Francesco; McCullough, Matthew; Thaler, Jesse

    2013-01-01

    Hints in the Fermi data for a 130 GeV gamma line from the galactic center have ignited interest in potential gamma line signatures of dark matter. Explanations of this line based on dark matter annihilation face a parametric tension since they often rely on large enhancements of loop-suppressed cross sections. In this paper, we pursue an alternative possibility that dark matter gamma lines could arise from ''semi-annihilation'' among multiple dark sector states. The semi-annihilation reaction ψ i ψ j → ψ k γ with a single final state photon is typically enhanced relative to ordinary annihilation ψ i ψ-bar i → γγ into photon pairs. Semi-annihilation allows for a wide range of dark matter masses compared to the fixed mass value required by annihilation, opening the possibility to explain potential dark matter signatures at higher energies. The most striking prediction of semi-annihilation is the presence of multiple gamma lines, with as many as order N 3 lines possible for N dark sector states, allowing for dark sector spectroscopy. A smoking gun signature arises in the simplest case of degenerate dark matter, where a strong semi-annihilation line at 130 GeV would be accompanied by a weaker annihilation line at 173 GeV. As a proof of principle, we construct two explicit models of dark matter semi-annihilation, one based on non-Abelian vector dark matter and the other based on retrofitting Rayleigh dark matter

  12. D-brane scattering and annihilation

    International Nuclear Information System (INIS)

    D’Amico, Guido; Gobbetti, Roberto; Kleban, Matthew; Schillo, Marjorie

    2015-01-01

    We study the dynamics of parallel brane-brane and brane-antibrane scattering in string theory in flat spacetime, focusing on the pair production of open strings that stretch between the branes. We are particularly interested in the case of scattering at small impact parameter bannihilating, so long as g s is small and the relative velocity v is neither too small nor too close to 1. Our analysis is relevant also to the case of charged open string production in world-volume electric fields, and we make use of this T-dual scenario in our analysis. We briefly discuss the application of our results to a stringy model of inflation involving moving branes.

  13. Characterization of lacunar defects by positrons annihilation

    CERN Document Server

    Barthe, M F; Blondiaux, G

    2003-01-01

    Among the nondestructive methods for the study of matter, the positrons annihilation method allows to sound the electronic structure of materials by measuring the annihilation characteristics. These characteristics depend on the electronic density as seen by the positon, and on the electron momentums distribution which annihilate with the positon. The positon is sensible to the coulombian potential variations inside a material and sounds preferentially the regions away from nuclei which represent potential wells. The lacunar-type defects (lack of nuclei) represent deep potential wells which can trap the positon up to temperatures close to the melting. This article describes the principles of this method and its application to the characterization of lacunar defects: 1 - positrons: matter probes (annihilation of electron-positon pairs, annihilation characteristics, positrons sources); 2 - positrons interactions in solids (implantation profiles, annihilation states, diffusion and trapping, positon lifetime spec...

  14. Positron annihilation in the interstellar medium

    Science.gov (United States)

    Guessoum, Nidhal; Ramaty, Reuven; Lingenfelter, Richard E.

    1991-01-01

    Positronium formation and annihilation are studied in a model for the interstellar medium consisting of cold cloud cores, warm partially ionized cloud envelopes, and hot intercloud gas. The gamma-ray spectra resulting from positron annihilation in these components of the interstellar medium are calculated. The spectra from the individual components are then combined, using two limiting assumptions for the propagation of the positrons, namely, that the positrons propagate freely throughout the interstellar medium, and that the positrons are excluded from the cold cloud cores. In the first case, the bulk of the positrons annihilate in the cloud cores and the annihilation line exhibits broad wings resulting from the annihilation of positronium formed by charge exchange in flight. In the second case, the positrons annihilate mainly in the warm envelopes, and the line wings are suppressed.

  15. Production bias and cluster annihilation: Why necessary?

    DEFF Research Database (Denmark)

    Singh, B.N.; Trinkaus, H.; Woo, C.H.

    1994-01-01

    the primary cluster density is high. Therefore, a sustained high swelling rate driven by production bias must involve the annihilation of primary clusters at sinks. A number of experimental observations which are unexplainable in terms of the conventional dislocation bias for monointerstitials is considered....... It is found that the production bias and cluster annihilation are necessary to explain these observations, with, in many cases, the explicit consideration of the annihilation of the primary interstitial clusters....

  16. Multimode vibrational couplings in resonant positron annihilation.

    Science.gov (United States)

    d'A Sanchez, Sergio; Lima, Marco A P; Varella, Márcio T do N

    2011-09-02

    The mechanisms for multimode vibrational couplings in resonant positron annihilation are not well understood. We show that these resonances can arise from positron-induced distortions of the potential energy surface (target response to the positron field). Though these distortions can transfer energy into single- and multiquantum vibrations, they have so far been disregarded as a pathway to resonant annihilation. We also compare the existing annihilation theories and show that the currently accepted model can be cast as a special case of the Feshbach annihilation theory.

  17. Use of X-ray diffraction, molecular simulations, and spectroscopy to determine the molecular packing in a polymer-fullerene bimolecular crystal

    KAUST Repository

    Miller, Nichole Cates

    2012-09-05

    The molecular packing in a polymer: fullerene bimolecular crystal is determined using X-ray diffraction (XRD), molecular mechanics (MM) and molecular dynamics (MD) simulations, 2D solid-state NMR spectroscopy, and IR absorption spectroscopy. The conformation of the electron-donating polymer is significantly disrupted by the incorporation of the electron-accepting fullerene molecules, which introduce twists and bends along the polymer backbone and 1D electron-conducting fullerene channels. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  18. Positron annihilation in solids: positronium diffusion; Annihilation du positon dans les solides diffusion du positonium

    Energy Technology Data Exchange (ETDEWEB)

    Paulin, R. [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires

    1969-04-01

    The existence of two slow components in life-time spectrum of positron annihilation in silicium, aluminium and alkaline-earth oxides powders is established. These two long mean-lives {approx_equal} 10{sup -9} s and {approx_equal} 10{sup -7} s result from annihilation, inside and outside the grains respectively, of ortho-positronium formed in defects present in ionic crystals investigated. Dynamic behaviour of Ps, so revealed, is analyzed in terms of diffusion in excellent agreement with experiment. Diffusion constants of the order of 10{sup -4} cm{sup 2} sec{sup -1} and mean path before annihilation from 50 to 300 Angstrom are measured. From 100 to 500 K the temperature influence upon diffusion process is effective only in SiO{sub 2} where activation energy is found about 10{sup -2} eV. The p-Ps zero point energy evaluated by angular correlation gives the order of magnitude for defects dimensions and diffusion mean-time. Finally, o-Ps behaviour in space between grains, where its interaction with atmospheric gases can be only detected, is analysed. (author) [French] Nous mettons en evidence l'existence de deux composantes lentes dans le spectre de temps de vie du positon avant annihilation dans des poudres d'oxydes alcalinoterreux d'alumine et de silice. Ces deux longues vies moyennes {approx_equal} 10{sup -9} s et {approx_equal} 10{sup -7} s resultent respectivement de l'annihilation a l'interieur et a l'exterieur des grains de l'ortho-positonium forme dans certains defauts presents dans les cristaux ioniques etudies. L'analyse des proprietes dynamiques du Ps ainsi revelees, est effectuee en termes de diffusion en excellent accord avec l'experience. Des constantes de diffusion de l'ordre de 10{sup -4} cm{sup 2} sec{sup -1} et des parcours moyens avant annihilation variant de 50 a 300 Angstrom sont ainsi mesures. Entre 100 et 500 K l'influence de la temperature sur le processus de diffusion n'est sensible

  19. Characterization of dynamics in complex lyophilized formulations: II. Analysis of density variations in terms of glass dynamics and comparisons with global mobility, fast dynamics, and Positron Annihilation Lifetime Spectroscopy (PALS)

    OpenAIRE

    Chieng, Norman; Cicerone, Marcus T.; Zhong, Qin; Liu, Ming; Pikal, Michael J.

    2013-01-01

    Amorphous HES/disaccharide (trehalose or sucrose) formulations, with and without added polyols (glycerol and sorbitol) and disaccharide formulations of human growth hormone (hGH), were prepared by freeze drying and characterized with particular interest in methodology for using high precision density measurements to evaluate free volume changes and a focus on comparisons between “free volume” changes obtained from analysis of density data, fast dynamics (local mobility), and PALS characteriza...

  20. Characterization of dynamics in complex lyophilized formulations: II. Analysis of density variations in terms of glass dynamics and comparisons with global mobility, fast dynamics, and Positron Annihilation Lifetime Spectroscopy (PALS)

    Science.gov (United States)

    Chieng, Norman; Cicerone, Marcus T.; Zhong, Qin; Liu, Ming; Pikal, Michael J.

    2013-01-01

    Amorphous HES/disaccharide (trehalose or sucrose) formulations, with and without added polyols (glycerol and sorbitol) and disaccharide formulations of human growth hormone (hGH), were prepared by freeze drying and characterized with particular interest in methodology for using high precision density measurements to evaluate free volume changes and a focus on comparisons between “free volume” changes obtained from analysis of density data, fast dynamics (local mobility), and PALS characterization of “free volume” hole size. Density measurements were performed using a helium gas pycnometer, and fast dynamics was characterized using incoherent neutron scattering spectrometer. Addition of sucrose and trehalose to hGH decreases free volume in the system with sucrose marginally more effective than trehalose, consistent with superior pharmaceutical stability of sucrose hGH formulations well below Tg relative to trehalose. We find that density data may be analyzed in terms of free volume changes by evaluation of volume changes on mixing and calculation of apparent specific volumes from the densities. Addition of sucrose to HES decreases free volume, but the effect of trehalose is not detectable above experimental error. Addition of sorbitol or glycerol to HES/trehalose base formulations appears to significantly decrease free volume, consistent with the positive impact of such additions on pharmaceutical stability (i.e., degradation) in the glassy state. Free volume changes, evaluated from density data, fast dynamics amplitude of local motion, and PALS hole size data generally are in qualitative agreement for the HES/disaccharide systems studied. All predict decreasing molecular mobility as disaccharides are added to HES. Global mobility as measured by enthalpy relaxation times, increases as disaccharides, particularly sucrose, are added to HES. PMID:23623797

  1. Characterization of dynamics in complex lyophilized formulations: II. Analysis of density variations in terms of glass dynamics and comparisons with global mobility, fast dynamics, and Positron Annihilation Lifetime Spectroscopy (PALS).

    Science.gov (United States)

    Chieng, Norman; Cicerone, Marcus T; Zhong, Qin; Liu, Ming; Pikal, Michael J

    2013-10-01

    Amorphous HES/disaccharide (trehalose or sucrose) formulations, with and without added polyols (glycerol and sorbitol) and disaccharide formulations of human growth hormone (hGH), were prepared by freeze drying and characterized with particular interest in methodology for using high precision density measurements to evaluate free volume changes and a focus on comparisons between "free volume" changes obtained from analysis of density data, fast dynamics (local mobility), and PALS characterization of "free volume" hole size. Density measurements were performed using a helium gas pycnometer, and fast dynamics was characterized using incoherent neutron scattering spectrometer. Addition of sucrose and trehalose to hGH decreases free volume in the system with sucrose marginally more effective than trehalose, consistent with superior pharmaceutical stability of sucrose hGH formulations well below Tg relative to trehalose. We find that density data may be analyzed in terms of free volume changes by evaluation of volume changes on mixing and calculation of apparent specific volumes from the densities. Addition of sucrose to HES decreases free volume, but the effect of trehalose is not detectable above experimental error. Addition of sorbitol or glycerol to HES/trehalose base formulations appears to significantly decrease free volume, consistent with the positive impact of such additions on pharmaceutical stability (i.e., degradation) in the glassy state. Free volume changes, evaluated from density data, fast dynamics amplitude of local motion, and PALS hole size data generally are in qualitative agreement for the HES/disaccharide systems studied. All predict decreasing molecular mobility as disaccharides are added to HES. Global mobility as measured by enthalpy relaxation times, increases as disaccharides, particularly sucrose, are added to HES. Copyright © 2013 Elsevier B.V. All rights reserved.

  2. Simple picture of the annihilation process

    International Nuclear Information System (INIS)

    Gotsman, E.; Nussinov, S.

    1980-01-01

    We propose a simple geometrical picture for B-barB annihilations, which is motivated by the electric-flux-tube model and is consistent with the quark-rearrangement model, as well as the nonplanar multiperipheral quark-exchange model. Within its framework we are able to explain all the salient features of the experimental annihilation data

  3. Positron annihilation in gamma-ray bursts

    Science.gov (United States)

    Harding, Alice K.

    1990-01-01

    Emission features appear at energies of 350 to 450 keV in the spectra of a number of gamma ray burst sources. These features were interpreted as electron-positron annihilation lines, redshifted by the gravitational field near the surface of a neutron star. Evidence that gamma ray bursts originate at neutron stars with magnetic field strengths of approx. 10(exp 12) Gauss came from recent observations of cyclotron scattering harmonics in the spectra of two bursts. Positrons could be produced in gamma ray burst sources either by photon-photon pair production or by one-photon pair production in a strong magnetic field. The annihilation of positrons is affected by the presence of a strong neutron star magnetic field in several ways. The relaxation of transverse momentum conservation causes an intrinsic broadening of the two-photon annihilation line and there is a decrease in the annihilation cross section below the free-space value. An additional channel for one-photon annihilation also becomes possible in high magnetic fields. The physics of pair production and annihilation near strongly magnetized neutron stars will be reviewed. Results from a self-consistent model for non-thermal synchrotron radiation and pair annihilation are beginning to identify the conditions required to produce observable annihilation features from strongly magnetized plasmas.

  4. WIMP Annihilation and Cooling of Neutron Stars

    DEFF Research Database (Denmark)

    Kouvaris, Christoforos

    2007-01-01

    We study the effect of WIMP annihilation on the temperature of a neutron star. We shall argue that the released energy due to WIMP annihilation inside the neutron stars, might affect the temperature of stars older than 10 million years, flattening out the temperature at $\\sim 10^4$ K for a typical...

  5. Positron annihilation characterization of nanostructured ferritic alloys

    International Nuclear Information System (INIS)

    Alinger, M.J.; Glade, S.C.; Wirth, B.D.; Odette, G.R.; Toyama, T.; Nagai, Y.; Hasegawa, M.

    2009-01-01

    Nanostructured ferritic alloys (NFAs) were produced by mechanically alloying Fe-14Cr-3W-0.4Ti and 0.25Y 2 O 3 (wt%) powders followed by hot isostatic pressing consolidation at 850, 1000 and 1150 deg. C. Positron annihilation lifetime and orbital momentum spectroscopy measurements are in qualitative agreement with small angle neutron scattering, transmission electron microscopy and atom probe tomography observations, indicating that up to 50% of the annihilations occur at high densities of Y-Ti-O enriched nm-scale features (NFs). Some annihilations may also occur in small cavities. In Y-free control alloys, that do not contain NFs, positrons primarily annihilate in the Fe-Cr matrix and at features such as dislocations, while a small fraction annihilate in large cavities or Ar bubbles.

  6. Recent advances in quantum scattering calculations on polyatomic bimolecular reactions.

    Science.gov (United States)

    Fu, Bina; Shan, Xiao; Zhang, Dong H; Clary, David C

    2017-12-11

    This review surveys quantum scattering calculations on chemical reactions of polyatomic molecules in the gas phase published in the last ten years. These calculations are useful because they provide highly accurate information on the dynamics of chemical reactions which can be compared in detail with experimental results. They also serve as quantum mechanical benchmarks for testing approximate theories which can more readily be applied to more complicated reactions. This review includes theories for calculating quantities such as rate constants which have many important scientific applications.

  7. Positron annihilation in transparent ceramics

    International Nuclear Information System (INIS)

    Husband, P; Selim, F A; Bartošová, I; Slugeň, V

    2016-01-01

    Transparent ceramics are emerging as excellent candidates for many photonic applications including laser, scintillation and illumination. However achieving perfect transparency is essential in these applications and requires high technology processing and complete understanding for the ceramic microstructure and its effect on the optical properties. Positron annihilation spectroscopy (PAS) is the perfect tool to study porosity and defects. It has been applied to investigate many ceramic structures; and transparent ceramics field may be greatly advanced by applying PAS. In this work positron lifetime (PLT) measurements were carried out in parallel with optical studies on yttrium aluminum garnet transparent ceramics in order to gain an understanding for their structure at the atomic level and its effect on the transparency and light scattering. The study confirmed that PAS can provide useful information on their microstructure and guide the technology of manufacturing and advancing transparent ceramics. (paper)

  8. Ultrafast Photoinduced Electron Transfer in Bimolecular Donor-Acceptor Systems

    KAUST Repository

    Alsulami, Qana A.

    2016-11-30

    The efficiency of photoconversion systems, such as organic photovoltaic (OPV) cells, is largely controlled by a series of fundamental photophysical processes occurring at the interface before carrier collection. A profound understanding of ultrafast interfacial charge transfer (CT), charge separation (CS), and charge recombination (CR) is the key determinant to improving the overall performances of photovoltaic devices. The discussion in this dissertation primarily focuses on the relevant parameters that are involved in photon absorption, exciton separation, carrier transport, carrier recombination and carrier collection in organic photovoltaic devices. A combination of steady-state and femtosecond broadband transient spectroscopies was used to investigate the photoinduced charge carrier dynamics in various donor-acceptor systems. Furthermore, this study was extended to investigate some important factors that influence charge transfer in donor-acceptor systems, such as the morphology, energy band alignment, electronic properties and chemical structure. Interestingly, clear correlations among the steady-state measurements, time-resolved spectroscopy results, grain alignment of the electron transporting layer (ETL), carrier mobility, and device performance are found. In this thesis, we explored the significant impacts of ultrafast charge separation and charge recombination at donor/acceptor (D/A) interfaces on the performance of a conjugated polymer PTB7-Th device with three fullerene acceptors: PC71BM, PC61BM and IC60BA. Time-resolved laser spectroscopy and high-resolution electron microscopy can illustrate the basis for fabricating solar cell devices with improved performances. In addition, we studied the effects of the incorporation of heavy metals into π-conjugated chromophores on electron transfer by monitoring the triplet state lifetime of the oligomer using transient absorption spectroscopy, as understanding the mechanisms controlling intersystem crossing and

  9. Mapping of exciton-exciton annihilation in MEH-PPV by time-resolved spectroscopy: experiment and microscopic theory.

    Science.gov (United States)

    Hader, Kilian; Consani, Cristina; Brixner, Tobias; Engel, Volker

    2017-12-06

    Transient absorption traces taken on samples of the polymer MEH-PPV are measured as a function of the laser intensity. In increasing the laser power, different decay dynamics of the signal are obtained. This suggests that effective exciton-exciton annihilation takes place. The signals are interpreted using a microscopic quantum mechanical model. The analysis points at an ultrafast excitonic decay via interchain and intrachain annihilation, where the latter process is roughly thirty times slower. Afterwards, diffusion-induced annihilation and relaxation become effective and thus determine the long-time behavior of the excited-state decay.

  10. Positron annihilation at grain boundaries in metals

    Czech Academy of Sciences Publication Activity Database

    Kuriplach, J.; Melikhova, O.; Hou, M.; Van Petegem, S.; Zhurkin, E.; Šob, Mojmír

    2007-01-01

    Roč. 4, č. 10 (2007), s. 3461-3464 ISSN 1862-6351. [International Conference on Positron Annihilation /14./. Hamilton, Ontario, 23.07.2006-28.07.2006] R&D Projects: GA AV ČR IAA1041302; GA MŠk OC 147 Institutional research plan: CEZ:AV0Z20410507 Keywords : positron annihilation * grain boundaries * electronic structure Subject RIV: BM - Solid Matter Physics ; Magnetism

  11. Soliton creation, propagation, and annihilation in aeromechanical arrays of one-way coupled bistable elements

    Science.gov (United States)

    Rosenberger, Tessa; Lindner, John F.

    We study the dynamics of mechanical arrays of bistable elements coupled one-way by wind. Unlike earlier hydromechanical unidirectional arrays, our aeromechanical one-way arrays are simpler, easier to study, and exhibit a broader range of phenomena. Soliton-like waves propagate in one direction at speeds proportional to wind speeds. Periodic boundaries enable solitons to annihilate in pairs in even arrays where adjacent elements are attracted to opposite stable states. Solitons propagate indefinitely in odd arrays where pairing is frustrated. Large noise spontaneously creates soliton- antisoliton pairs, as predicted by prior computer simulations. Soliton annihilation times increase quadratically with initial separations, as expected for random walk models of soliton collisions.

  12. Turing instability and bifurcation analysis in a diffusive bimolecular system with delayed feedback

    Science.gov (United States)

    Wei, Xin; Wei, Junjie

    2017-09-01

    A diffusive autocatalytic bimolecular model with delayed feedback subject to Neumann boundary conditions is considered. We mainly study the stability of the unique positive equilibrium and the existence of periodic solutions. Our study shows that diffusion can give rise to Turing instability, and the time delay can affect the stability of the positive equilibrium and result in the occurrence of Hopf bifurcations. By applying the normal form theory and center manifold reduction for partial functional differential equations, we investigate the stability and direction of the bifurcations. Finally, we give some simulations to illustrate our theoretical results.

  13. Positron Cooling and Annihilation in Noble Gases.

    Science.gov (United States)

    Green, D G

    2017-11-17

    Positron cooling and annihilation in room temperature noble gases is simulated using accurate scattering and annihilation cross sections calculated with many-body theory, enabling the first simultaneous probing of the energy dependence of the scattering and annihilation cross sections. A strikingly small fraction of positrons is shown to survive to thermalization: ∼0.1 in He, ∼0 in Ne, ∼0.15 in Ar, ∼0.05 in Kr, and ∼0.01 in Xe. For Xe, the time-varying annihilation rate Z[over ¯]_{eff}(τ) is shown to be highly sensitive to the depletion of the momentum distribution due to annihilation, conclusively explaining the long-standing discrepancy between gas-cell and trap-based measurements. Overall, the use of the accurate atomic data gives Z[over ¯]_{eff}(τ) in close agreement with experiment for all noble gases except Ne, the experiment for which is proffered to have suffered from incomplete knowledge of the fraction of positrons surviving to thermalization and/or the presence of impurities.

  14. Positron annihilation induced Auger electron spectroscopy

    Science.gov (United States)

    Weiss, Alex; Koymen, A. R.; Mehl, David; Jensen, K. O.; Lei, Chun; Lee, K. H.

    1990-01-01

    Recently, Weiss et al. have demonstrated that it is possible to excite Auger transitions by annihilating core electrons using a low energy (less than 30eV) beam of positrons. This mechanism makes possible a new electron spectroscopy, Positron annihilation induced Auger Electron Spectroscopy (PAES). The probability of exciting an Auger transition is proportional to the overlap of the positron wavefunction with atomic core levels. Since the Auger electron energy provides a signature of the atomic species making the transition, PAES makes it possible to determine the overlap of the positron wavefunction with a particular element. PAES may therefore provide a means of detecting positron-atom complexes. Measurements of PAES intensities from clean and adsorbate covered Cu surfaces are presented which indicate that approx. 5 percent of positrons injected into CU at 25eV produce core annihilations that result in Auger transitions.

  15. Radiative corrections to neutralino annihilation. Recent developments

    International Nuclear Information System (INIS)

    Herrmann, Bjoern

    2010-11-01

    Evaluating the relic density of dark matter is an interesting possibility to constrain the parameter space of new physics models. However, this calculation is affected by several sources of uncertainty. On the particle physics side, considerable progress has been made in the recent years concerning the calculation of the annihilation cross-section of dark matter, which is needed in this context. In particular, within the Minimal Supersymmetric Standard Model, the theoretical uncertainty has been reduced through the calculation of loop corrections. The present contribution gives an overview over the achievements that have been made in QCD corrections to neutralino pair annihilation. The numerical impact is illustrated for a few examples. (orig.)

  16. Energy-resolved positron annihilation for molecules

    International Nuclear Information System (INIS)

    Barnes, L.D.; Gilbert, S.J.; Surko, C.M.

    2003-01-01

    This paper presents an experimental study designed to address the long-standing question regarding the origin of very large positron annihilation rates observed for many molecules. We report a study of the annihilation, resolved as a function of positron energy (ΔE∼25 meV, full width at half maximum) for positron energies from 50 meV to several eV. Annihilation measurements are presented for a range of hydrocarbon molecules, including a detailed study of alkanes, C n H 2n+2 , for n=1-9 and 12. Data for other molecules are also presented: C 2 H 2 , C 2 H 4 ; CD 4 ; isopentane; partially fluorinated and fluorinated methane (CH x F 4-x ); 1-fluorohexane (C 6 H 13 F) and 1-fluorononane (C 9 H 19 F). A key feature of the results is very large enhancements in the annihilation rates at positron energies corresponding to the excitation of molecular vibrations in larger alkane molecules. These enhancements are believed to be responsible for the large annihilation rates observed for Maxwellian distributions of positrons in molecular gases. In alkane molecules larger than ethane (C 2 H 6 ), the position of these peaks is shifted downward by an amount ∼20 meV per carbon. The results presented here are generally consistent with a physical picture recently considered in detail by Gribakin [Phys. Rev. A 61, 022720 (2000)]. In this model, the incoming positron excites a vibrational Feshbach resonance and is temporarily trapped on the molecule, greatly enhancing the probability of annihilation. The applicability of this model and the resulting enhancement in annihilation rate relies on the existence of positron-molecule bound states. In accord with this reasoning, the experimental results presented here provide the most direct evidence to date that positrons bind to neutral molecules. The shift in the position of the resonances is interpreted as a measure of the binding energy of the positron to the molecule. Other features of the results are also discussed, including large

  17. Porous silicon investigated by positron annihilation

    International Nuclear Information System (INIS)

    Cruz, R.M. de la; Pareja, R.

    1989-01-01

    The effect of the anodic conversion in silicon single crystals is investigated by positron lifetime measurements. Anodization at constant current induces changes in the positron lifetime spectrum of monocrystalline silicon samples. It is found that theses changes are primarily dependent on the silicon resistivity. The annihilation parameter behaviour of anodized samples, treated at high temperature under reducing conditions, is also investigated. The results reveal that positron annihilation can be a useful technique to characterize porous silicon formed by anodizing as well as to investigate its thermal behaviour. (author)

  18. Inverse Compton Gamma Rays from Dark Matter Annihilation in the ...

    Indian Academy of Sciences (India)

    Electron spectrum as a function of electron energy for three different values of Mχ annihilating into b¯b final state. the annihilation cross sections are obtained from Ackermann et al. (2014). The DM annihilation takes place predominantly through some combination of the final states b¯b, tt, W. +. W. − or ZZ. The gamma ray ...

  19. Vortex annihilation and inverse cascades in two dimensional superfluid turbulence

    Science.gov (United States)

    Lucas, Andrew; Chesler, Paul M.

    2015-03-01

    The dynamics of a dilute mixture of vortices and antivortices in a turbulent two-dimensional superfluid at finite temperature is well described by first order Hall-Vinen-Iordanskii equations, or dissipative point vortex dynamics. These equations are governed by a single dimensionless parameter: the ratio of the strength of drag forces to Magnus forces on vortices. When this parameter is small, we demonstrate using numerical simulations that the resulting superfluid enjoys an inverse energy cascade where small scale stirring leads to large scale vortex clustering. We argue analytically and numerically that the vortex annihilation rate in a laminar flow may be parametrically smaller than the rate in a turbulent flow with an inverse cascade. This suggests a new way to detect inverse cascades in experiments on two-dimensional superfluid turbulence using cold atomic gases, where traditional probes of turbulence such as the energy spectrum are not currently accessible.

  20. A positron annihilation study of hydrated DNA

    DEFF Research Database (Denmark)

    Warman, J. M.; Eldrup, Morten Mostgaard

    1986-01-01

    Positron annihilation measurements are reported for hydrated DNA as a function of water content and as a function of temperature (20 to -180.degree. C) for samples containing 10 and 50% wt of water. The ortho-positronium mean lifetime and its intensity show distinct variations with the degree of ...

  1. PAES: Positron annihilation induced Auger electron spectrometer

    Directory of Open Access Journals (Sweden)

    Christoph Hugenschmidt

    2015-08-01

    Full Text Available Positron annihilation induced Auger electron spectroscopy (PAES is a newly developed application for surface studies with high elemental selectivity and exceptional surface sensitivity. The instrument is operated by the Technische Universität München and is located at NEPOMUC.

  2. A positron annihilation study of hydrated DNA

    DEFF Research Database (Denmark)

    Warman, J. M.; Eldrup, Morten Mostgaard

    1986-01-01

    Positron annihilation measurements are reported for hydrated DNA as a function of water content and as a function of temperature (20 to -180.degree. C) for samples containing 10 and 50% wt of water. The ortho-positronium mean lifetime and its intensity show distinct variations with the degree...

  3. Nondestructive examination using neutron activated positron annihilation

    Science.gov (United States)

    Akers, Douglas W.; Denison, Arthur B.

    2001-01-01

    A method is provided for performing nondestructive examination of a metal specimen using neutron activated positron annihilation wherein the positron emitter source is formed within the metal specimen. The method permits in situ nondestructive examination and has the advantage of being capable of performing bulk analysis to determine embrittlement, fatigue and dislocation within a metal specimen.

  4. Positron annihilation radiation from the Galactic center region

    Science.gov (United States)

    Ramaty, R.; Lingenfelter, R. E.

    1991-01-01

    Observations show that there are two components of positron annihilation radiation from the region of the Galactic center: a variable component resulting from one or just a few compact sources at or near the Galactic center and a steady, diffuse component resulting from positron annihilation in the Galactic disk. The diffuse component is modeled using the observed longitude distributions of 70-150 MeV gamma rays, CO, and hot plasma revealed by Fe line emission. Recent results on positron annihilation in the interstellar medium are reviewed and the implications of the annihilation processes on the fraction of positrons annihilating via positronium and on the shape of the 511 keV annihilation line are discussed. The sources of diffuse Galactic positrons are also reviewed and the nature of the compact source of annihilation radiation near the Galactic center is discussed.

  5. Simplified Representation of Partial and Total Rate Constants of Complex-Forming Bimolecular Reactions.

    Science.gov (United States)

    Troe, J

    2015-12-17

    The temperature and pressure dependence of partial and total rate constants of complex-forming bimolecular reactions are investigated with the goal to obtain simplified and compact rate constant expressions suitable for data compilations. The transition of the reactions from low pressure chemical activation to high pressure association character is analyzed. The two processes are modeled separately first by solving master equations, leading to "inverse" and "normal" falloff curves, respectively, and allowing for a compact representation of the separated rate constants. It is shown that broadening factors of the two falloff curves are different, and those of chemical activation often approaching unity. Coupling of the two separate processes then is modeled in a simplified manner. Finally, thermal redissociation of the adducts formed by association is accounted for.

  6. Searching for dark matter annihilation in the Smith high-velocity cloud

    International Nuclear Information System (INIS)

    Drlica-Wagner, Alex; Gómez-Vargas, Germán A.; Hewitt, John W.; Linden, Tim; Tibaldo, Luigi

    2014-01-01

    Recent observations suggest that some high-velocity clouds may be confined by massive dark matter halos. In particular, the proximity and proposed dark matter content of the Smith Cloud make it a tempting target for the indirect detection of dark matter annihilation. We argue that the Smith Cloud may be a better target than some Milky Way dwarf spheroidal satellite galaxies and use γ-ray observations from the Fermi Large Area Telescope to search for a dark matter annihilation signal. No significant γ-ray excess is found coincident with the Smith Cloud, and we set strong limits on the dark matter annihilation cross section assuming a spatially extended dark matter profile consistent with dynamical modeling of the Smith Cloud. Notably, these limits exclude the canonical thermal relic cross section (∼ 3 × 10 –26 cm 3 s –1 ) for dark matter masses ≲ 30 GeV annihilating via the b b-bar or τ + τ – channels for certain assumptions of the dark matter density profile; however, uncertainties in the dark matter content of the Smith Cloud may significantly weaken these constraints.

  7. Searching for dark matter annihilation in the Smith high-velocity cloud

    Energy Technology Data Exchange (ETDEWEB)

    Drlica-Wagner, Alex [Center for Particle Astrophysics, Fermi National Accelerator Laboratory, Batavia, IL 60510 (United States); Gómez-Vargas, Germán A. [Departamento de Fisíca, Pontificia Universidad Católica de Chile, Avenida Vicuña Mackenna 4860, Santiago (Chile); Hewitt, John W. [CRESST, University of Maryland, Baltimore County, Baltimore, MD 21250 (United States); Linden, Tim [The Kavli Institute for Cosmological Physics, University of Chicago, Chicago, IL 60637 (United States); Tibaldo, Luigi [W. W. Hansen Experimental Physics Laboratory, Kavli Institute for Particle Astrophysics and Cosmology, Department of Physics and SLAC National Accelerator Laboratory, Stanford University, Stanford, CA 94305 (United States)

    2014-07-20

    Recent observations suggest that some high-velocity clouds may be confined by massive dark matter halos. In particular, the proximity and proposed dark matter content of the Smith Cloud make it a tempting target for the indirect detection of dark matter annihilation. We argue that the Smith Cloud may be a better target than some Milky Way dwarf spheroidal satellite galaxies and use γ-ray observations from the Fermi Large Area Telescope to search for a dark matter annihilation signal. No significant γ-ray excess is found coincident with the Smith Cloud, and we set strong limits on the dark matter annihilation cross section assuming a spatially extended dark matter profile consistent with dynamical modeling of the Smith Cloud. Notably, these limits exclude the canonical thermal relic cross section (∼ 3 × 10{sup –26} cm{sup 3} s{sup –1}) for dark matter masses ≲ 30 GeV annihilating via the b b-bar or τ{sup +}τ{sup –} channels for certain assumptions of the dark matter density profile; however, uncertainties in the dark matter content of the Smith Cloud may significantly weaken these constraints.

  8. Searching for Dark Matter Annihilation in the Smith High-Velocity Cloud

    Science.gov (United States)

    Drlica-Wagner, Alex; Gomez-Vargas, German A.; Hewitt, John W.; Linden, Tim; Tibaldo, Luigi

    2014-01-01

    Recent observations suggest that some high-velocity clouds may be confined by massive dark matter halos. In particular, the proximity and proposed dark matter content of the Smith Cloud make it a tempting target for the indirect detection of dark matter annihilation. We argue that the Smith Cloud may be a better target than some Milky Way dwarf spheroidal satellite galaxies and use gamma-ray observations from the Fermi Large Area Telescope to search for a dark matter annihilation signal. No significant gamma-ray excess is found coincident with the Smith Cloud, and we set strong limits on the dark matter annihilation cross section assuming a spatially extended dark matter profile consistent with dynamical modeling of the Smith Cloud. Notably, these limits exclude the canonical thermal relic cross section (approximately 3 x 10 (sup -26) cubic centimeters per second) for dark matter masses less than or approximately 30 gigaelectronvolts annihilating via the B/B- bar oscillation or tau/antitau channels for certain assumptions of the dark matter density profile; however, uncertainties in the dark matter content of the Smith Cloud may significantly weaken these constraints.

  9. Positron Annihilation in the Undergraduate Laboratory

    Science.gov (United States)

    Engbrecht, Jason

    2017-04-01

    While there are a variety of undergraduate laboratory experiments in the literature, they tend to focus on specific positron experiments and use specialized equipment that limit their flexibility. Here we present a positron spectroscopy experimental apparatus designed for the undergraduate lab. Rather than specialized pulse processing the apparatus utilizes a PC oscilloscope as its primary data acquisition utility with pulse processing happening in software instead of hardware. This allows the apparatus to explore a variety of physical phenomena with the positron annihilation including material science, 2 and 3 gamma annihilation properties, polarimetry via Compton scattering, QED tests, and local hidden variable theories. The supporting software is flexible and allows students to pursue these experiments through exploration rather than simply supporting data acquisition. St. Olaf College.

  10. Two photon annihilation operators and squeezed vacuum

    Science.gov (United States)

    Roy, Anil K.; Mehta, C. L.; Saxena, G. M.

    1993-01-01

    Inverses of the harmonic oscillator creation and annihilation operators by their actions on the number states are introduced. Three of the two photon annihilation operators, viz., a(sup +/-1)a, aa(sup +/-1), and a(sup 2), have normalizable right eigenstates with nonvanishing eigenvalues. The eigenvalue equation of these operators are discussed and their normalized eigenstates are obtained. The Fock state representation in each case separates into two sets of states, one involving only the even number states while the other involving only the odd number states. It is shown that the even set of eigenstates of the operator a(sup +/-1)a is the customary squeezed vacuum S(sigma) O greater than.

  11. Method for photon activation positron annihilation analysis

    Science.gov (United States)

    Akers, Douglas W.

    2006-06-06

    A non-destructive testing method comprises providing a specimen having at least one positron emitter therein; determining a threshold energy for activating the positron emitter; and determining whether a half-life of the positron emitter is less than a selected half-life. If the half-life of the positron emitter is greater than or equal to the selected half-life, then activating the positron emitter by bombarding the specimen with photons having energies greater than the threshold energy and detecting gamma rays produced by annihilation of positrons in the specimen. If the half-life of the positron emitter is less then the selected half-life, then alternately activating the positron emitter by bombarding the specimen with photons having energies greater then the threshold energy and detecting gamma rays produced by positron annihilation within the specimen.

  12. A possible signature of annihilating dark matter

    Science.gov (United States)

    Chan, Man Ho

    2018-02-01

    In this article, we report a new signature of dark matter annihilation based on the radio continuum data of NGC 1569 galaxy detected in the past few decades. After eliminating the thermal contribution of the radio signal, an abrupt change in the spectral index is shown in the radio spectrum. Previously, this signature was interpreted as an evidence of convective outflow of cosmic ray. However, we show that the cosmic ray contribution is not enough to account for the observed radio flux. We then discover that if dark matter annihilates via the 4-e channel with the thermal relic cross-section, the electrons and positrons produced would emit a strong radio flux which can provide an excellent agreement with the observed signature. The best-fitting dark matter mass is 25 GeV.

  13. Revisiting the annihilation decay anti Bs→π+π-

    International Nuclear Information System (INIS)

    Yang, Yadong; Su, Fang; Lu, Gongru; Hao, Hongjun

    2005-01-01

    It is very important to know the strength of the annihilation contribution in B charmless non-leptonic decays. The anti B s →π + π - process could serve as a good probe of the strength. We have studied the process in the QCD factorization framework. Using a gluon mass scale dictated by the studies of infrared behavior of gluon propagators to avoid enhancements in the soft endpoint regions, we find that the CP averaged branching ratio is about 1.24 x 10 -7 , the direct CP asymmetry C ππ is about -0.05, while the mixing-induced CP asymmetry is quite large with the value S ππ =0.18. This process could be measured at LHC-b experiments in the near future and would deepen our understanding of the dynamics of B charmless decays. (orig.)

  14. Overlapping resonances in e+e- annihilation

    International Nuclear Information System (INIS)

    Dothan, Y.; Horn, D.

    1976-06-01

    The application of the general formalism of two overlapping resonances to the inclusive process of hadron production in e + e - annihilation is discussed. The strong dip observed near 4 GeV can be fitted by three different classes of solutions, all of which have to use an overlap close to its maximal value. This suggests that both resonances have one common main decay channel. The implications of this conclusion are briefly discussed

  15. Systems of branching, annihilating, and coalescing particles

    Czech Academy of Sciences Publication Activity Database

    Athreya, S. R.; Swart, Jan M.

    2012-01-01

    Roč. 17, č. 80 (2012), s. 1-32 ISSN 1083-6489 R&D Projects: GA ČR GAP201/10/0752 Institutional support: RVO:67985556 Keywords : reaction-diffusion process * branching * coalescence * annihilation * thinning * Poissonization Subject RIV: BA - General Mathematics Impact factor: 0.785, year: 2012 http://library.utia.cas.cz/separaty/2012/SI/swart-0381108.pdf

  16. Positron annihilation spectroscopy in condensed matter

    International Nuclear Information System (INIS)

    Brauer, G.

    1982-09-01

    The topic of positron annihilation spectroscopy (PAS) is the investigation of all aspects connected with the annihilation of slow positrons. This work deals with the application of PAS to different problems of materials science. The first chapter is an introduction to fundamental aspects of positron annihilation, as far as they are important to the different experimental techniques of PAS. Chapter 2 is concerned with the information obtainable by PAS. The three main experimental techniques of PAS (2γ-angular correlation, positron lifetime and Doppler broadening) are explained and problems in the application of these methods are discussed. Chapter 3 contains experimental results. According to the different fields of application it was subgrouped into: 1. Investigations of crystalline solids. Detection of structural defects in Cu, estimation of defect concentrations, study of the sintering of Cu powders as well as lattice defects in V 3 Si. 2. Chemical investigations. Structure of mixed solvents, selective solvation of mixed solvents by electrolytes as well as the micellization of sodium dodecylsulphate in aqueous solutions. 3. Investigations of glasses. Influence of heat treatment and production technology on the preorder of X-amorphous silica glass as well as preliminary measurements of pyrocerams. 4. Investigations of metallic glasses. Demonstration of the influence of production technology on parameters measurable by PAS. Chapter 4 contains a summary as well as an outlook of further applications of PAS to surface physics, medicine, biology and astrophysics. (author)

  17. Pair creation, motion, and annihilation of topological defects in two-dimensional nematic liquid crystals

    Science.gov (United States)

    Cortese, Dario; Eggers, Jens; Liverpool, Tanniemola B.

    2018-02-01

    We present a framework for the study of disclinations in two-dimensional active nematic liquid crystals and topological defects in general. The order tensor formalism is used to calculate exact multiparticle solutions of the linearized static equations inside a planar uniformly aligned state so that the total charge has to vanish. Topological charge conservation then requires that there is always an equal number of q =1 /2 and q =-1 /2 charges. Starting from a set of hydrodynamic equations, we derive a low-dimensional dynamical system for the parameters of the static solutions, which describes the motion of a half-disclination pair or of several pairs. Within this formalism, we model defect production and annihilation, as observed in experiments. Our dynamics also provide an estimate for the critical density at which production and annihilation rates are balanced.

  18. Initial angular momentum state in pp annihilation at rest

    CERN Document Server

    Bizzarri, R

    1972-01-01

    The author shows that no quantitative statement on the relative importance of initial P-states in pp annihilation can be made. Annihilations in flight indicate that P-wave annihilation into K/sub 1 //sup 0/K/sub 1//sup 0/ is inhibited while annihilation into pi pi is enhanced and might suggest a P-wave contamination approximately 10%. The observatory of the final state K/sub 1//sup 0/K/sub 1//sup 0/n from annihilations at rest indicates that the depression of the K/sub 1//sup 0/K/sub 1//sup 0/ final state is not so important and suggests a P-wave contamination smaller than 4%. Furthermore the successes obtained in the analysis of various final states on the assumption of S-wave annihilation are hard to reconcile with a P-wave contribution bigger than approximately 5%. (20 refs).

  19. ANTICOOL: Simulating positron cooling and annihilation in atomic gases

    Science.gov (United States)

    Green, D. G.

    2018-03-01

    The Fortran program ANTICOOL, developed to simulate positron cooling and annihilation in atomic gases for positron energies below the positronium-formation threshold, is presented. Given positron-atom elastic scattering phase shifts, normalised annihilation rates Zeff, and γ spectra as a function of momentum k, ANTICOOL enables the calculation of the positron momentum distribution f(k , t) as a function of time t, the time-varying normalised annihilation rate Z¯eff(t) , the lifetime spectrum and time-varying annihilation γ spectra. The capability and functionality of the program is demonstrated via a tutorial-style example for positron cooling and annihilation in room temperature helium gas, using accurate scattering and annihilation cross sections and γ spectra calculated using many-body theory as input.

  20. Trojan War displayed as a full annihilation-diffusion-reaction model

    Science.gov (United States)

    Flores, J. C.

    2017-02-01

    The diffusive pair annihilation model with embedded topological domains and archaeological data is applied in an analysis of the hypothetical Trojan-Greek war during the late Bronze Age. Estimations of parameter are explicitly made for critical dynamics of the model. In particular, the 8-metre walls of Troy could be viewed as the effective shield that provided the technological difference between the two armies. Suggestively, the numbers in The Iliad are quite sound, being in accord with Lanchester's laws of warfare.

  1. Bimolecular Coupling as a Vector for Decomposition of Fast-Initiating Olefin Metathesis Catalysts.

    Science.gov (United States)

    Bailey, Gwendolyn A; Foscato, Marco; Higman, Carolyn S; Day, Craig S; Jensen, Vidar R; Fogg, Deryn Elizabeth

    2018-04-13

    The correlation between rapid initiation and rapid decomposition in olefin metathesis is probed for a series of fast-initiating Ru catalysts: the Hoveyda catalyst HII, RuCl2(L)(=CHC6H4-o-OiPr); the Grela catalyst nG (a derivative of HII with a nitro group para to OiPr); the Piers catalyst PII, [RuCl2(L)(=CHPCy3)]OTf; the third-generation Grubbs catalyst GIII, RuCl2(L)(py)2(=CHPh); and dianiline catalyst DA, RuCl2(L)(o-dianiline)(=CHPh) (L = H2IMes = N,N'-bis (mesityl)-imidazolin-2-ylidene). Prior studies of ethylene metathesis established that various Ru metathesis catalysts can decompose by -elimination of propene from metallacyclobutane RuCl2(H2IMes)(2-C3H6) Ru-2. The present work demonstrates that in metathesis of terminal olefins, -elimination yields only ca. 25-40% propenes for HII, nG, PII or DA, and none for GIII. The discrepancy is attributed to competing decomposition via bimolecular coupling of methylidene intermediate RuCl2(H2IMes)(=CH2) Ru-1. Direct evidence for methylidene coupling is presented, via the controlled decomposition of transiently-stabilized adducts of Ru-1, RuCl2(H2IMes)Ln(=CH2) (Ln = pyn'; n' = 1, 2, or o-dianiline). These adducts were synthesized by treating in situ-generated metallacyclobutane Ru-2 with pyridine or o-dianiline, and isolated at low temperature (-116 °C or -78 °C, respectively). On warming, both undergo methylidene coupling, liberating ethylene and forming RuCl2(H2IMes)Ln. A mechanism is proposed based on kinetic studies and molecular-level computational analysis. Bimolecular coupling emerges as an important contributor to the instability of Ru-1, and a potentially major pathway for decomposition of fast-initiating, phosphine-free metathesis catalysts.

  2. Development of bimolecular fluorescence complementation using rsEGFP2 for detection and super-resolution imaging of protein-protein interactions in live cells.

    Science.gov (United States)

    Wang, Sheng; Ding, Miao; Chen, Xuanze; Chang, Lei; Sun, Yujie

    2017-06-01

    Direct visualization of protein-protein interactions (PPIs) at high spatial and temporal resolution in live cells is crucial for understanding the intricate and dynamic behaviors of signaling protein complexes. Recently, bimolecular fluorescence complementation (BiFC) assays have been combined with super-resolution imaging techniques including PALM and SOFI to visualize PPIs at the nanometer spatial resolution. RESOLFT nanoscopy has been proven as a powerful live-cell super-resolution imaging technique. With regard to the detection and visualization of PPIs in live cells with high temporal and spatial resolution, here we developed a BiFC assay using split rsEGFP2, a highly photostable and reversibly photoswitchable fluorescent protein previously developed for RESOLFT nanoscopy. Combined with parallelized RESOLFT microscopy, we demonstrated the high spatiotemporal resolving capability of a rsEGFP2-based BiFC assay by detecting and visualizing specifically the heterodimerization interactions between Bcl-x L and Bak as well as the dynamics of the complex on mitochondria membrane in live cells.

  3. Bimolecular Excited-State Electron Transfer with Surprisingly Long-Lived Radical Ions

    KAUST Repository

    Alsam, Amani Abdu

    2015-09-02

    We explored the excited-state interactions of bimolecular, non-covalent systems consisting of cationic poly[(9,9-di(3,3’-N,N’-trimethyl-ammonium) propyl fluorenyl-2,7-diyl)-alt-co-(9,9-dioctyl-fluorenyl-2,7-diyl)] diiodide salt (PFN) and 1,4-dicyanobenzene (DCB) using steady-state and time-resolved techniques, including femto- and nanosecond transient absorption and femtosecond infrared spectroscopies with broadband capabilities. The experimental results demonstrated that photo-induced electron transfer from PFN to DCB occurs on the picosecond time scale, leading to the formation of PFN+• and DCB-• radical ions. Interestingly, real-time observations of the vibrational marker modes on the acceptor side provided direct evidence and insight into the electron transfer process indirectly inferred from UV-Vis experiments. The band narrowing on the picosecond time scale observed on the antisymmetric C-N stretching vibration of the DCB radical anion provides clear experimental evidence that a substantial part of the excess energy is channeled into vibrational modes of the electron transfer product and that the geminate ion pairs dissociate. More importantly, our nanosecond time-resolved data indicate that the charge-separated state is very long lived ( 30 ns) due to the dissociation of the contact radical ion pair into free ions. Finally, the fast electron transfer and slow charge recombination anticipate the current donor−acceptor system with potential applications in organic solar cells.

  4. Real-time observation of intersystem crossing induced by charge recombination during bimolecular electron transfer reactions

    KAUST Repository

    Alsam, Amani Abdu

    2016-09-21

    Real-time probing of intersystem crossing (ISC) and triplet-state formation after photoinduced electron transfer (ET) is a particularly challenging task that can be achieved by time-resolved spectroscopy with broadband capability. Here, we examine the mechanism of charge separation (CS), charge recombination (CR) and ISC of bimolecular photoinduced electron transfer (PET) between poly[(9,9-di(3,3′-N,N’-trimethyl-ammonium) propyl fluorenyl-2,7-diyl)-alt-co-(9,9-dioctyl-fluorenyl-2,7-diyl)] diiodide salt (PFN) and dicyanobenzene (DCB) using time-resolved spectroscopy. PET from PFN to DCB is confirmed by monitoring the transient absorption (TA) and infrared spectroscopic signatures for the radical ion pair (DCB─•-PFN+•). In addition, our time-resolved results clearly demonstrate that CS takes place within picoseconds followed by CR within nanoseconds. The ns-TA data exhibit the clear spectroscopic signature of PFN triplet-triplet absorption, induced by the CR of the radical ion pairs (DCB─•-PFN+•). As a result, the triplet state of PFN (3PFN*) forms and subsequently, the ground singlet state is replenished within microseconds. © 2016

  5. Interactions among the early Escherichia coli divisome proteins revealed by bimolecular fluorescence complementation.

    Science.gov (United States)

    Pazos, Manuel; Natale, Paolo; Margolin, William; Vicente, Miguel

    2013-12-01

    We used bimolecular fluorescence complementation (BiFC) assays to detect protein-protein interactions of all possible pairs of the essential Escherichia coli proto-ring components, FtsZ, FtsA and ZipA, as well as the non-essential FtsZ-associated proteins ZapA and ZapB. We found an unexpected interaction between ZipA and ZapB at potential cell division sites, and when co-overproduced, they induced long narrow constrictions at division sites that were dependent on FtsZ. These assays also uncovered an interaction between ZipA and ZapA that was mediated by FtsZ. BiFC with ZapA and ZapB showed that in addition to their expected interaction at midcell, they also interact at the cell poles. BiFC detected interaction between FtsZ and ZapB at midcell and close to the poles. Results from the remaining pairwise combinations confirmed known interactions between FtsZ and ZipA, and ZapB with itself. © 2013 Society for Applied Microbiology and John Wiley & Sons Ltd.

  6. Formulation and Evaluation of CTRW Governing Equations for Irreversible, Bimolecular Reactions During Transport

    Science.gov (United States)

    Hansen, S. K.; Berkowitz, B.

    2014-12-01

    The continuous time random walk (CTRW) formalism is a valuable tool for modeling both conservative and reversibly sorbing solute transport in heterogeneous porous media, underpinning both Eulerian (integrodifferential equation-based) and Lagrangian (particle tracking) approaches to transport modeling. More recently, there has been interest in modeling transport with irreversible reactions, and Lagrangian CTRW-based numerical models have been successfully applied to these problems. However, a corresponding Eulerian theory has been lacking. We recently developed Eulerian governing equations in the presence of irreversible bimolecular reactions, via the device of upscaling transport and treating reactions at a finer scale. The technique is generally valid, even in porous media that do not have an obvious division of length scales, subject to certain smoothness assumptions on the solution. We show that the governing equations we develop simplify, under appropriate circumstances, to both the generalized master equation for the unreactive CTRW and to the advection-dispersion-reaction equation. We also present a numerical corroboration of our development and its underlying smoothness assumptions obtained using a novel, indirect particle-tracking / partial differential equation hybrid technique. We discuss the implications of the new governing equations for practical reactive transport modeling and for conceptualization of subsurface processes, and highlight connections to other approaches. As applicable, we will also discuss aspects of numerical implementation.

  7. ESI-MS Investigation of an Equilibrium between a Bimolecular Quadruplex DNA and a Duplex DNA/RNA Hybrid.

    Science.gov (United States)

    Birrento, Monica L; Bryan, Tracy M; Samosorn, Siritron; Beck, Jennifer L

    2015-07-01

    Electrospray ionization mass spectrometry (ESI-MS) conditions were optimized for simultaneous observation of a bimolecular qDNA and a Watson-Crick base-paired duplex DNA/RNA hybrid. The DNA sequence used was telomeric DNA, and the RNA contained the template for telomerase-mediated telomeric DNA synthesis. Addition of RNA to the quadruplex DNA (qDNA) resulted in formation of the duplex DNA/RNA hybrid. Melting profiles obtained using circular dichroism spectroscopy confirmed that the DNA/RNA hybrid exhibited greater thermal stability than the bimolecular qDNA in solution. Binding of a 13-substituted berberine (1) derivative to the bimolecular qDNA stabilized its structure as evidenced by an increase in its stability in the mass spectrometer, and an increase in its circular dichroism (CD) melting temperature of 10°C. The DNA/RNA hybrid did not bind the ligand extensively and its thermal stability was unchanged in the presence of (1). The qDNA-ligand complex resisted unfolding in the presence of excess RNA, limiting the formation of the DNA/RNA hybrid. Previously, it has been proposed that DNA secondary structures, such as qDNA, may be involved in the telomerase mechanism. DNA/RNA hybrid structures occur at the active site of telomerase. The results presented in the current work show that if telomeric DNA was folded into a qDNA structure, it is possible for a DNA/RNA hybrid to form as is required during template alignment. The discrimination of ligand (1) for binding to the bimolecular qDNA over the DNA/RNA hybrid positions it as a useful compound for probing the role(s), if any, of antiparallel qDNA in the telomerase mechanism.

  8. Dark Matter Annihilation at the Galactic Center

    Energy Technology Data Exchange (ETDEWEB)

    Linden, Timothy Ryan [Univ. of California, Santa Cruz, CA (United States)

    2013-06-01

    Observations by the WMAP and PLANCK satellites have provided extraordinarily accurate observations on the densities of baryonic matter, dark matter, and dark energy in the universe. These observations indicate that our universe is composed of approximately ve times as much dark matter as baryonic matter. However, e orts to detect a particle responsible for the energy density of dark matter have been unsuccessful. Theoretical models have indicated that a leading candidate for the dark matter is the lightest supersymmetric particle, which may be stable due to a conserved R-parity. This dark matter particle would still be capable of interacting with baryons via weak-force interactions in the early universe, a process which was found to naturally explain the observed relic abundance of dark matter today. These residual annihilations can persist, albeit at a much lower rate, in the present universe, providing a detectable signal from dark matter annihilation events which occur throughout the universe. Simulations calculating the distribution of dark matter in our galaxy almost universally predict the galactic center of the Milky Way Galaxy (GC) to provide the brightest signal from dark matter annihilation due to its relative proximity and large simulated dark matter density. Recent advances in telescope technology have allowed for the rst multiwavelength analysis of the GC, with suitable e ective exposure, angular resolution, and energy resolution in order to detect dark matter particles with properties similar to those predicted by the WIMP miracle. In this work, I describe ongoing e orts which have successfully detected an excess in -ray emission from the region immediately surrounding the GC, which is di cult to describe in terms of standard di use emission predicted in the GC region. While the jury is still out on any dark matter interpretation of this excess, I describe several related observations which may indicate a dark matter origin. Finally, I discuss the

  9. Annihilation model of the Tormac sheath

    International Nuclear Information System (INIS)

    Hammer, J.H.

    1979-02-01

    A one-dimensional, steady state fluid model is developed to describe the boundary layer between plasma and magnetic field that occurs in the Tormac sheath. Similar systems which may be treatable by the same model are tokamaks with divertors and reversed field mirrors. The model includes transport across the magnetic field as well as mirror losses along the field, the latter being represented as annihilation terms in the one-dimensional equations. The model equations are derived from the two-dimensional, time dependent hierarchy of equations generated by taking velocity moments of the kinetic equation including collisions

  10. On baryogenesis from dark matter annihilation

    International Nuclear Information System (INIS)

    Bernal, Nicolás; Colucci, Stefano; Ubaldi, Lorenzo; Josse-Michaux, François-Xavier; Racker, J.

    2013-01-01

    We study in detail the conditions to generate the baryon asymmetry of the universe from the annihilation of dark matter. This scenario requires a low energy mechanism for thermal baryogenesis, hence we first discuss some of these mechanisms together with the specific constraints due to the connection with the dark matter sector. Then we show that, contrary to what stated in previous studies, it is possible to generate the cosmological asymmetry without adding a light sterile dark sector, both in models with violation and with conservation of B−L. In addition, one of the models we propose yields some connection to neutrino masses

  11. From creation and annihilation operators to statistics

    Science.gov (United States)

    Hoyuelos, M.

    2018-01-01

    A procedure to derive the partition function of non-interacting particles with exotic or intermediate statistics is presented. The partition function is directly related to the associated creation and annihilation operators that obey some specific commutation or anti-commutation relations. The cases of Gentile statistics, quons, Polychronakos statistics, and ewkons are considered. Ewkons statistics was recently derived from the assumption of free diffusion in energy space (Hoyuelos and Sisterna, 2016); an ideal gas of ewkons has negative pressure, a feature that makes them suitable for the description of dark energy.

  12. Jets in e+e- annihilation

    International Nuclear Information System (INIS)

    Hanson, G.G.

    1978-05-01

    The latest results on R, the ratio of the total cross section for production of multihadronic events to the muon pair production cross section, and inclusive distributions of hadrons from e + e - annihilation in the center-of-mass energy range from 2.6 to 7.8 GeV are presented. The evidence for jet structure is reviewed. Inclusive distributions of hadrons in Feynman x, rapidity, and transverse momentum relative to the jet direction are studied. Particular emphasis is placed on the method used to measure these inclusive distributions and the biases which might result from this method

  13. Particle-antiparticle asymmetries from annihilations.

    Science.gov (United States)

    Baldes, Iason; Bell, Nicole F; Petraki, Kalliopi; Volkas, Raymond R

    2014-10-31

    An extensively studied mechanism to create particle-antiparticle asymmetries is the out-of-equilibrium and CP violating decay of a heavy particle. We, instead, examine how asymmetries can arise purely from 2→2 annihilations rather than from the usual 1→2 decays and inverse decays. We review the general conditions on the reaction rates that arise from S-matrix unitarity and CPT invariance, and show how these are implemented in the context of a simple toy model. We formulate the Boltzmann equations for this model, and present an example solution.

  14. Apparatus for photon activation positron annihilation analysis

    Science.gov (United States)

    Akers, Douglas W [Idaho Falls, ID

    2007-06-12

    Non-destructive testing apparatus according to one embodiment of the invention comprises a photon source. The photon source produces photons having predetermined energies and directs the photons toward a specimen being tested. The photons from the photon source result in the creation of positrons within the specimen being tested. A detector positioned adjacent the specimen being tested detects gamma rays produced by annihilation of positrons with electrons. A data processing system operatively associated with the detector produces output data indicative of a lattice characteristic of the specimen being tested.

  15. New particles produced in electron--positron annihilation

    International Nuclear Information System (INIS)

    Perl, M.L.

    1975-01-01

    The main properties of the new particles produced in e + e - annihilation are reviewed. Included are properties of the continuum region, the 4.1-GeV enhancement, the psi and psi', radiative decays of the psi and psi', singly charmed particle searches in e + - e - annihilation, and the e/sub μ/ events

  16. Study of double scattering effect in antiproton--deuteron annihilation

    International Nuclear Information System (INIS)

    Zemany, P.D.

    1975-01-01

    The double scattering process in the deuteron is investigated for the reaction anti pd → p/sub s/ + mesons. About 30 percent of the apparent anti pn annihilations are involved in double scattering. A model which describes the properties of protons emerging from apparent anti pn annihilations is presented

  17. Soliton annihilation in the perturbed sine-Gordon system

    DEFF Research Database (Denmark)

    Pedersen, Niels Falsig; Samuelsen, Mogens Rugholm; Welner, D.

    1984-01-01

    Fluxon-antifluxon annihilation in the perturbed sine-Gordon equation with loss and driving terms is investigated. For the infinite line we find a simple analytic expression for the threshold driving term corresponding to annihilation. With the application of the results to a Josephson junction of...

  18. Impact of dark matter decays and annihilations on structure formation

    NARCIS (Netherlands)

    Mapelli, M.; Ripamonti, E.

    2007-01-01

    Abstract: We derived the evolution of the energy deposition in the intergalactic medium (IGM) by different decaying (or annihilating) dark matter (DM) candidates. Heavy annihilating DM particles (with mass larger than a few GeV) have no influence on reionization and heating, even if we assume that

  19. CMB constraint on dark matter annihilation after Planck 2015

    Energy Technology Data Exchange (ETDEWEB)

    Kawasaki, Masahiro [Institute for Cosmic Ray Research, The University of Tokyo, Kashiwa, Chiba 277-8568 (Japan); Kavli IPMU (WPI), UTIAS, The University of Tokyo, Kashiwa, Chiba 277-8583 (Japan); Nakayama, Kazunori, E-mail: kazunori@hep-th.phys.s.u-tokyo.ac.jp [Department of Physics, Faculty of Science, The University of Tokyo, Bunkyo-ku, Tokyo 133-0033 (Japan); Kavli IPMU (WPI), UTIAS, The University of Tokyo, Kashiwa, Chiba 277-8583 (Japan); Sekiguchi, Toyokazu [Institute for Basic Science, Center for Theoretical Physics of the Universe, Daejeon 34051 (Korea, Republic of)

    2016-05-10

    We update the constraint on the dark matter annihilation cross section by using the recent measurements of the CMB anisotropy by the Planck satellite. We fully calculate the cascade of dark matter annihilation products and their effects on ionization, heating and excitation of the hydrogen, hence do not rely on any assumption on the energy fractions that cause these effects.

  20. Nucleon-antinucleon annihilation in chiral soliton model

    International Nuclear Information System (INIS)

    Musakhanov, M.M.; Tashkentskij Gosudarstvennyj Univ., Tashkent; Musatov, I.V.

    1991-01-01

    We investigate annihilation process of nucleons in the chiral soliton model by the path integral method. A soliton-antisoliton pair is shown to decay into mesons at range of about 1fm, defined by the S bar S potential. Contribution of the annihilation channel to the elastic scattering is discussed

  1. Studies of defects and defect agglomerates by positron annihilation spectroscopy

    DEFF Research Database (Denmark)

    Eldrup, Morten Mostgaard; Singh, B.N.

    1997-01-01

    A brief introduction to positron annihilation spectroscopy (PAS), and in particular lo its use for defect studies in metals is given. Positrons injected into a metal may become trapped in defects such as vacancies, vacancy clusters, voids, bubbles and dislocations and subsequently annihilate from...

  2. Positron annihilation studies of neutron irradiated reactor pressure vessel steels

    International Nuclear Information System (INIS)

    Brauer, G.; Liszkay, L.; Molnar, B.

    1988-01-01

    Several annealing studies by positron annihilation (Doppler broadening, lifetime) on neutron irradiated Cr-Mo-V reactor pressure vessel steels (Soviet type 15Kh2MFA) regarding the influences of irradiation temperature, fluence of fast neutrons as well as different impurity contents are presented and discussed. A possibility of explaining the positron annihilation data by irradiation induced carbide formation is proposed. (author)

  3. CMB constraint on dark matter annihilation after Planck 2015

    Directory of Open Access Journals (Sweden)

    Masahiro Kawasaki

    2016-05-01

    Full Text Available We update the constraint on the dark matter annihilation cross section by using the recent measurements of the CMB anisotropy by the Planck satellite. We fully calculate the cascade of dark matter annihilation products and their effects on ionization, heating and excitation of the hydrogen, hence do not rely on any assumption on the energy fractions that cause these effects.

  4. Direct evidence for positron annihilation from shallow traps

    DEFF Research Database (Denmark)

    Linderoth, Søren; Hidalgo, C.

    1987-01-01

    For deformed Ag the temperature dependence of the positron lifetime parameters is followed between 12 and 300 K. Clear direct evidence for positron trapping and annihilation at shallow traps, with a positron binding energy of 9±2 meV and annihilation characteristics very similar to those...

  5. The Antiproton-Nucleon Annihilation Process (Antiproton Collaboration Experiment)

    Science.gov (United States)

    Barkas, W. H.; Birge, R. W.; Chupp, W. W.; Ekspong, A. G.; Goldhaber, G.; Goldhaber, S.; Heckman, H. H.; Perkins, D. H.; Sandweiss, J.; Segre, E.; Smith, F. M.; Stork, D. H.; Rossum, L. Van; Amaldi, E.; Baroni, G.; Castagnoli, C.; Franzinetti, C.; Manfredini, A.

    1956-09-10

    In the exposure to a 700-MeV/c negative particle beam, 35 antiproton stars have been found. Of these antiprotons, 21 annihilate in flight and three give large-angle scatters ({Theta} > 15 , T{sub P-} > 50 Mev), while 14 annihilate at rest. From the interactions in flight we obtain the total cross section for antiproton interaction.

  6. Identification of effective exciton-exciton annihilation in squaraine-squaraine copolymers.

    Science.gov (United States)

    Hader, Kilian; May, Volkhard; Lambert, Christoph; Engel, Volker

    2016-05-11

    Ultrafast time-resolved transient absorption spectroscopy is able to monitor the fate of the excited state population in molecular aggregates or polymers. Due to many competing decay processes, the identification of exciton-exciton annihilation (EEA) is difficult. Here, we use a microscopic model to describe exciton annihilation processes in squaraine-squaraine copolymers. Transient absorption time traces measured at different laser powers exhibit an unusual time-dependence. The analysis points towards dynamics taking place on three time-scales. Immediately after laser-excitation a localization of excitons takes place within the femtosecond time-regime. This is followed by exciton-exciton annihilation which is responsible for a fast decay of the exciton population. At later times, excitations being localized on units which are not directly connected remain so that diffusion dominates the dynamics and leads to a slower decay. We thus provide evidence for EEA tracked by time-resolved spectroscopy which has not been reported that clearly before.

  7. Local electron-electron interaction strength in ferromagnetic nickel determined by spin-polarized positron annihilation.

    Science.gov (United States)

    Ceeh, Hubert; Weber, Josef Andreas; Weber, Josef Andreass; Böni, Peter; Leitner, Michael; Benea, Diana; Chioncel, Liviu; Ebert, Hubert; Minár, Jan; Vollhardt, Dieter; Hugenschmidt, Christoph

    2016-02-16

    We employ a positron annihilation technique, the spin-polarized two-dimensional angular correlation of annihilation radiation (2D-ACAR), to measure the spin-difference spectra of ferromagnetic nickel. The experimental data are compared with the theoretical results obtained within a combination of the local spin density approximation (LSDA) and the many-body dynamical mean-field theory (DMFT). We find that the self-energy defining the electronic correlations in Ni leads to anisotropic contributions to the momentum distribution. By direct comparison of the theoretical and experimental results we determine the strength of the local electronic interaction U in ferromagnetic Ni as 2.0 ± 0.1 eV.

  8. Triplet-triplet annihilation upconversion kinetics of C60-Bodipy dyads as organic triplet photosensitizers.

    Science.gov (United States)

    Wei, Yaxiong; Zhou, Miaomiao; Zhou, Qiaohui; Zhou, Xiaoguo; Liu, Shilin; Zhang, Song; Zhang, Bing

    2017-08-23

    Three new triplet photosensitizers consisting of a bodipy derivative and C 60 moieties were synthesized for triplet-triplet annihilation upconversion of perylene. With the extension of the π-conjugated structure of the bodipy derivative, the three photosensitizers exhibited different absorption wavelengths, e.g. 517 nm for B-2, 532 nm for B-4, and 557 nm for B-6. The steady-state and transient absorption, steady-state fluorescence, and upconverted fluorescence emission were investigated to reveal step-by-step the dynamic processes of the above systems. The quantum yields of intramolecular energy transfer, intersystem crossing, and triplet-triplet energy transfer were measured. From the upconverted fluorescence emission spectra, the overall quantum yield of the triplet-triplet annihilation upconversion, Φ UC , was determined to be 5.80% for B-2, 7.95% for B-4, and 4.99% for B-6.

  9. Photochemical reaction dynamics

    Energy Technology Data Exchange (ETDEWEB)

    Moore, B.C. [Lawrence Berkeley Laboratory, Livermore, CA (United States)

    1993-12-01

    The purpose of the program is to develop a fundamental understanding of unimolecular and bimolecular reaction dynamics with application in combustion and energy systems. The energy dependence in ketene isomerization, ketene dissociation dynamics, and carbonyl substitution on organometallic rhodium complexes in liquid xenon have been studied. Future studies concerning unimolecular processes in ketene as well as energy transfer and kinetic studies of methylene radicals are discussed.

  10. Constraining annihilating dark matter by radio data of M33

    Science.gov (United States)

    Chan, Man Ho

    2017-08-01

    Recent studies of radio data put strong constraints on annihilation cross sections for dark matter. In this article, we provide the first analysis of using M33 radio data in constraining annihilating dark matter. The resulting constraints of annihilation cross sections for some channels are more stringent than that obtained from six years of Fermi Large Area Telescope (Fermi-LAT) gamma-ray observations of the Milky Way dwarf spheroidal satellite galaxies. In particular, the conservative lower limits of dark matter mass annihilating via e+e-, μ+μ- and τ+τ- channels are 190, 120 and 70 GeV, respectively, with the thermal relic annihilation cross section. These results are in significant tension with some of the recent quantitative analyses of the AMS-02 and Fermi-LAT data of the Milky Way center.

  11. Thermal equilibrium defects in anthracene probed by positron annihilation

    International Nuclear Information System (INIS)

    Uedono, Akira; Tanigawa, Shoichiro; Tachibana, Masaru; Shimizu, Mikio; Satoh, Masaaki; Kojima, Kenichi; Ishibashi, Shoji; Kawano, Takao.

    1996-01-01

    Defects in anthracene were investigated by the positron annihilation technique. Doppler broadening profiles of the annihilation radiation and lifetime spectra of positrons were measured in the temperature range between 305 K and 516 K. The lifetime of positrons annihilated from the delocalized state was determined to be 0.306 ns around room temperature. Below the melting point, the observed temperature dependence of the line shape parameter S was explained assuming the formation energy of thermal equilibrium defects was 1 eV. Above the melting point, the pick-off annihilation of ortho-positronium in open spaces was observed, where the size of these spaces was estimated to be 0.2 nm 3 . The annihilation of positrons from the self-trapped state was also discussed. (author)

  12. Thermal equilibrium defects in anthracene probed by positron annihilation

    Energy Technology Data Exchange (ETDEWEB)

    Uedono, Akira; Tanigawa, Shoichiro [Tsukuba Univ., Ibaraki (Japan). Inst. of Materials Science; Tachibana, Masaru; Shimizu, Mikio; Satoh, Masaaki; Kojima, Kenichi; Ishibashi, Shoji; Kawano, Takao

    1996-06-01

    Defects in anthracene were investigated by the positron annihilation technique. Doppler broadening profiles of the annihilation radiation and lifetime spectra of positrons were measured in the temperature range between 305 K and 516 K. The lifetime of positrons annihilated from the delocalized state was determined to be 0.306 ns around room temperature. Below the melting point, the observed temperature dependence of the line shape parameter S was explained assuming the formation energy of thermal equilibrium defects was 1 eV. Above the melting point, the pick-off annihilation of ortho-positronium in open spaces was observed, where the size of these spaces was estimated to be 0.2 nm{sup 3}. The annihilation of positrons from the self-trapped state was also discussed. (author)

  13. Positron annihilation in the nuclear outflows of the Milky Way

    Science.gov (United States)

    Panther, Fiona H.; Crocker, Roland M.; Birnboim, Yuval; Seitenzahl, Ivo R.; Ruiter, Ashley J.

    2018-02-01

    Observations of soft gamma rays emanating from the Milky Way from SPI/INTEGRAL reveal the annihilation of ˜2 × 1043 positrons every second in the Galactic bulge. The origin of these positrons, which annihilate to produce a prominent emission line centred at 511 keV, has remained mysterious since their discovery almost 50 yr ago. A plausible origin for the positrons is in association with the intense star formation ongoing in the Galactic centre. Moreover, there is strong evidence for a nuclear outflow in the Milky Way. We find that advective transport and subsequent annihilation of positrons in such an outflow cannot simultaneously replicate the observed morphology of positron annihilation in the Galactic bulge and satisfy the requirement that 90 per cent of positrons annihilate once the outflow has cooled to 104 K.

  14. First positron annihilation lifetime measurement of Pu

    International Nuclear Information System (INIS)

    Colmenares, C.; Howell, R.H.; Ancheta, D.; Cowan, T.; Hanafee, J.; Sterne, P.

    1996-01-01

    We have made the first measurement of defects in an aged sample of δ phase, Ga stabilized Pu, using positron annihilation lifetime spectroscopy. This measurement validates the procedure necessary to perform measurements on this highly toxic material and obtain data representative of sample conditions. Comparison of the positron annihilation lifetime analysis of the data with calculated values suggests that He filled vacancies or vacancy clusters dominate the defect population. Such defects are the necessary precursor to void growth and swelling. The evolution of defects resulting from the radioactive decay of Pu during its life in the stockpile is one of the unknown quantities affecting our confidence in predictions of the limit on stockpile components. Radiation damage leads to changes in the size and strength of metals studied for reactor and accelerator use and similar effects may be expected in Pu. The evolution of radiation produced vacancies into larger void structures and accompanying macroscopic swelling may occur in Pu at some age. A detailed understanding of the defects in self irradiated Pu is required to predict the time scale of void swelling and related radiation effects. 1 fig

  15. Modeling Bimolecular Reactions and Transport in Porous Media Via Particle Tracking

    Energy Technology Data Exchange (ETDEWEB)

    Dong Ding; David Benson; Amir Paster; Diogo Bolster

    2012-01-01

    We use a particle-tracking method to simulate several one-dimensional bimolecular reactive transport experiments. In this numerical method, the reactants are represented by particles: advection and dispersion dominate the flow, and molecular diffusion dictates, in large part, the reactions. The particle/particle reactions are determined by a combination of two probabilities dictated by the physics of transport and energetics of reaction. The first is that reactant particles occupy the same volume over a short time interval. The second is the conditional probability that two collocated particles favorably transform into a reaction. The first probability is a direct physical representation of the degree of mixing in an advancing displacement front, and as such lacks empirical parameters except for the user-defined number of particles. This number can be determined analytically from concentration autocovariance, if this type of data is available. The simulations compare favorably to two physical experiments. In one, the concentration of product, 1,2-naphthoquinoe-4-aminobenzene (NQAB) from reaction between 1,2-naphthoquinone-4-sulfonic acid (NQS) and aniline (AN), was measured at the outflow of a column filled with glass beads at different times. In the other, the concentration distribution of reactants (CuSO_4 and EDTA^{4-}) and products (CuEDTA^{4-}) were quantified by snapshots of transmitted light through a column packed with cryloite sand. The thermodynamic rate coefficient in the latter experiment was 10^7 times greater than the former experiment, making it essentially instantaneous. When compared to the solution of the advection-dispersion-reaction equation (ADRE) with the well-mixed reaction coefficient, the experiments and the particle-tracking simulations showed on the order of 20% to 40% less overall product, which is attributed to poor mixing. The poor mixing also leads to higher product concentrations on the edges of the mixing zones, which the particle

  16. Simulation of the annihilation emission of galactic positrons

    International Nuclear Information System (INIS)

    Gillard, W.

    2008-01-01

    Positrons annihilate in the central region of our Galaxy. This has been known since the detection of a strong emission line centered on an energy of 511 keV in the direction of the Galactic center. This gamma-ray line is emitted during the annihilation of positrons with electrons from the interstellar medium. The spectrometer SPI, onboard the INTEGRAL observatory, performed spatial and spectral analyses of the positron annihilation emission. This thesis presents a study of the Galactic positron annihilation emission based on models of the different interactions undergone by positrons in the interstellar medium. The models are relied on our present knowledge of the properties of the interstellar medium in the Galactic bulge, where most of the positrons annihilate, and of the physics of positrons (production, propagation and annihilation processes). In order to obtain constraints on the positrons sources and physical characteristics of the annihilation medium, we compared the results of the models to measurements provided by the SPI spectrometer. (author)

  17. Multi-photon creation and single-photon annihilation of electron-positron pairs

    International Nuclear Information System (INIS)

    Hu, Huayu

    2011-01-01

    In this thesis we study multi-photon e + e - pair production in a trident process, and singlephoton e + e - pair annihilation in a triple interaction. The pair production is considered in the collision of a relativistic electron with a strong laser beam, and calculated within the theory of laser-dressed quantum electrodynamics. A regularization method is developed systematically for the resonance problem arising in the multi-photon process. Total production rates, positron spectra, and relative contributions of different reaction channels are obtained in various interaction regimes. Our calculation shows good agreement with existing experimental data from SLAC, and adds further insights into the experimental findings. Besides, we study the process in a manifestly nonperturbative domain, whose accessibility to future all-optical experiments based on laser acceleration is shown. In the single-photon e + e - pair annihilation, the recoil momentum is absorbed by a spectator particle. Various kinematic configurations of the three incoming particles are examined. Under certain conditions, the emitted photon exhibits distinct angular and polarization distributions which could facilitate the detection of the process. Considering an equilibrium relativistic e + e - plasma, it is found that the single-photon process becomes the dominant annihilation channel for plasma temperatures above 3 MeV. Multi-particle correlation effects are therefore essential for the e + e - dynamics at very high density. (orig.)

  18. Multi-photon creation and single-photon annihilation of electron-positron pairs

    Energy Technology Data Exchange (ETDEWEB)

    Hu, Huayu

    2011-04-27

    In this thesis we study multi-photon e{sup +}e{sup -} pair production in a trident process, and singlephoton e{sup +}e{sup -} pair annihilation in a triple interaction. The pair production is considered in the collision of a relativistic electron with a strong laser beam, and calculated within the theory of laser-dressed quantum electrodynamics. A regularization method is developed systematically for the resonance problem arising in the multi-photon process. Total production rates, positron spectra, and relative contributions of different reaction channels are obtained in various interaction regimes. Our calculation shows good agreement with existing experimental data from SLAC, and adds further insights into the experimental findings. Besides, we study the process in a manifestly nonperturbative domain, whose accessibility to future all-optical experiments based on laser acceleration is shown. In the single-photon e{sup +}e{sup -} pair annihilation, the recoil momentum is absorbed by a spectator particle. Various kinematic configurations of the three incoming particles are examined. Under certain conditions, the emitted photon exhibits distinct angular and polarization distributions which could facilitate the detection of the process. Considering an equilibrium relativistic e{sup +}e{sup -} plasma, it is found that the single-photon process becomes the dominant annihilation channel for plasma temperatures above 3 MeV. Multi-particle correlation effects are therefore essential for the e{sup +}e{sup -} dynamics at very high density. (orig.)

  19. Study of radiation damage in metals by positron annihilation

    International Nuclear Information System (INIS)

    Gauster, W.B.

    1977-01-01

    Positron annihilation is a sensitive technique for probing defects in metals and it has recently been shown to be a valuable tool for the study of radiation damage. After an introduction to the three basic experimental methods (angular correlation, Doppler broadening, and lifetime measurements), the interaction of positrons with lattice defects is reviewed. Results for the annealing of damage after low temperature irradiation are used to show that positron annihilation has provided new information on annealing kinetics. The role of positron techniques in characterizing complex defect structures resulting from high-temperature neutron irradiation is reviewed and the possible utility of positron annihilation as a nondestructive monitor of property changes is pointed out

  20. Photoluminescence and positron annihilation spectroscopic investigation on a H(+) irradiated ZnO single crystal.

    Science.gov (United States)

    Sarkar, A; Chakrabarti, Mahuya; Sanyal, D; Bhowmick, D; Dechoudhury, S; Chakrabarti, A; Rakshit, Tamita; Ray, S K

    2012-08-15

    Low temperature photoluminescence and room temperature positron annihilation spectroscopy have been employed to investigate the defects incorporated by 6 MeV H(+) ions in a hydrothermally grown ZnO single crystal. Prior to irradiation, the emission from donor bound excitons is at 3.378 eV (10 K). The irradiation creates an intense and narrow emission at 3.368 eV (10 K). The intensity of this peak is nearly four times that of the dominant near band edge peak of the pristine crystal. The characteristic features of the 3.368 eV emission indicate its origin as a 'hydrogen at oxygen vacancy' type defect. The positron annihilation lifetime measurement reveals a single component lifetime spectrum for both the unirradiated (164 ± 1 ps) and irradiated crystal (175 ± 1 ps). It reflects the fact that the positron lifetime and intensity of the new irradiation driven defect species are a little higher compared to those in the unirradiated crystal. However, the estimated defect concentration, even considering the high dynamic defect annihilation rate in ZnO, comes out to be ∼4 × 10(17) cm(-3) (using SRIM software). This is a very high defect concentration compared to the defect sensitivity of positron annihilation spectroscopy. A probable reason is the partial filling of the incorporated vacancies (positron traps), which in ZnO are zinc vacancies. The positron lifetime of ∼175 ps (in irradiated ZnO) is consistent with recent theoretical calculations for partially hydrogen-filled zinc vacancies in ZnO. Passivation of oxygen vacancies by hydrogen is also reflected in the photoluminescence results. A possible reason for such vacancy filling (at both Zn and O sites) due to irradiation has also been discussed.

  1. Excited-state annihilation reduces power dependence of single-molecule FRET experiments.

    Science.gov (United States)

    Nettels, Daniel; Haenni, Dominik; Maillot, Sacha; Gueye, Moussa; Barth, Anders; Hirschfeld, Verena; Hübner, Christian G; Léonard, Jérémie; Schuler, Benjamin

    2015-12-28

    Single-molecule Förster resonance energy transfer (FRET) experiments are an important method for probing biomolecular structure and dynamics. The results from such experiments appear to be surprisingly independent of the excitation power used, in contradiction to the simple photophysical mechanism usually invoked for FRET. Here we show that excited-state annihilation processes are an essential cause of this behavior. Singlet-singlet annihilation (SSA) is a mechanism of fluorescence quenching induced by Förster-type energy transfer between two fluorophores while they are both in their first excited singlet states (S1S1), which is usually neglected in the interpretation of FRET experiments. However, this approximation is only justified in the limit of low excitation rates. We demonstrate that SSA is evident in fluorescence correlation measurements for the commonly used FRET pair Alexa 488/Alexa 594, with a rate comparable to the rate of energy transfer between the donor excited state and the acceptor ground state (S1S0) that is exploited in FRET experiments. Transient absorption spectroscopy shows that SSA occurs exclusively via energy transfer from Alexa 488 to Alexa 594. Excitation-power dependent microsecond correlation experiments support the conclusion based on previously reported absorption spectra of triplet states that singlet-triplet annihilation (STA) analogously mediates energy transfer if the acceptor is in the triplet state. The results indicate that both SSA and STA have a pronounced effect on the overall FRET process and reduce the power dependence of the observed FRET efficiencies. The existence of annihilation processes thus seems to be essential for using FRET as a reliable spectroscopic ruler at the high excitation rates commonly employed in single-molecule spectroscopy.

  2. Annihilation of vortex dipoles in an Oblate Bose-Einstein Condensate

    OpenAIRE

    Prabhakar, Shashi; Singh, R. P.; Gautam, S.; Angom, D.

    2011-01-01

    We theoretically explore the annihilation of vortex dipoles, generated when an obstacle moves through an oblate Bose-Einstein condensate, and examine the energetics of the annihilation event. We show that the gray soliton, which results from the vortex dipole annihilation, is lower in energy than the vortex dipole. We also investigate the annihilation events numerically and observe that the annihilation occurs only when the vortex dipole overtakes the obstacle and comes closer than the cohere...

  3. Gas phase studies of the Pesci decarboxylation reaction: synthesis, structure, and unimolecular and bimolecular reactivity of organometallic ions.

    Science.gov (United States)

    O'Hair, Richard A J; Rijs, Nicole J

    2015-02-17

    promoting the formation of the organometallic ion. Where isomeric organometallic ions are generated and normal MS approaches cannot distinguish them, we describe approaches to elucidate the decarboxylation mechanism via determination of their structure. These "unmasked" organometallic ions, [RM(L)n](x), can also be structurally interrogated spectroscopically or via CID. We have thus compared the gas-phase structures and decomposition of several highly reactive and synthetically important organometallic ions for the first time. Perhaps the most significant aspect of this work is the study of bimolecular reactions, which provides experimental information on mechanistically obscure bond-formation and cross-coupling steps and the intrinsic reactivity of ions. We have sought to understand transformations of substrates including acid-base and hydrolysis reactions, along with reactions resulting in C-C bond formation. Our studies also allow a direct comparison of the performance of different metal catalysts in the individual elementary steps associated with protodecarboxylation and decarboxylative alkylation cycles. Electronic structure (DFT and ab initio) and dynamics (RRKM) calculations provide further mechanistic insights into these reactions. The broad implications of this research are that new reactions can be discovered and that the performance of metal catalysts can be evaluated in terms of each of their elementary steps. This has been particularly useful for the study of metal-mediated decarboxylation reactions.

  4. Subliminal psychodynamic activation method and annihilation anxiety: preliminary findings.

    Science.gov (United States)

    Greenberg, A C

    1992-02-01

    Research with the subliminal psychodynamic activation (SPA) method has led to improvements in subjects' functioning in a variety of areas, including but not limited to weight control, school grades, and feelings of general anxiety. In 1987, Hurvich proposed that the SPA method could be used to further the understanding of annihilation anxiety. 100 nonclinical subjects completed questionnaires pertaining to annihilation anxiety, psychological differentiation, and state anxiety and were tachistoscopically exposed to the subliminal message of symbiotic-like oneness, MOMMY AND I ARE ONE, and to control messages. Analysis showed that women with low annihilation anxiety had significantly lower state anxiety than women with high annihilation anxiety, regardless of the content of the subliminal message; results did not reach significance for men. Correlations among scores on the questionnaires also were noted.

  5. Entanglement-annihilating and entanglement-breaking channels

    International Nuclear Information System (INIS)

    Moravcikova, Lenka; Ziman, Mario

    2010-01-01

    We introduce and investigate a family of entanglement-annihilating channels. These channels are capable of destroying any quantum entanglement within the system they act on. We show that they are not necessarily entanglement breaking. In order to achieve this result we analyze the subset of locally entanglement-annihilating channels. In this case, the same local noise applied on each subsystem individually is less entanglement annihilating (with respect to multi-partite entanglement) as the number of subsystems is increasing. Therefore, the bipartite case provides restrictions on the set of local entanglement-annihilating channels for the multipartite case. The introduced concepts are illustrated on the family of single-qubit depolarizing channels.

  6. φ production in anti pp annihilation at rest

    International Nuclear Information System (INIS)

    Reifenroether, J.; Beuchert, K.; Duch, K.D.; Kalinowsky, H.; Klempt, E.; May, B.; Weidenauer, P.; Gastaldi, U.; Landua, R.; Dahme, W.; Bizot, J.C.; Delcourt, B.; White, B.L.; Amsler, C.; Doser, M.; Riedlberger, J.; Straumann, U.; Truoel, P.

    1991-01-01

    We report on measurements of the branching ratios for φ production in anti pp annihilation at rest in H 2 gas. Branching ratios for φπ 0 , φη, φρ 0 , φω and φπ + π - are determined for two data sets with different contributions of annihilations from S and P states of the anti pp system. The branching ratios are compared to corresponding annihilation modes where the φ is replaced by an ω meson. We conclude that φ production is in most reactions enhanced with respect to the expectation based on the OZI rule. In annihilations from the spin triplet ground state of antiprotonic hydrogen into φπ the OZI rule is violated dramatically. (orig.)

  7. Black Hole Window into p-Wave Dark Matter Annihilation.

    Science.gov (United States)

    Shelton, Jessie; Shapiro, Stuart L; Fields, Brian D

    2015-12-04

    We present a new method to measure or constrain p-wave-suppressed cross sections for dark matter (DM) annihilations inside the steep density spikes induced by supermassive black holes. We demonstrate that the high DM densities, together with the increased velocity dispersion, within such spikes combine to make thermal p-wave annihilation cross sections potentially visible in γ-ray observations of the Galactic center (GC). The resulting DM signal is a bright central point source with emission originating from DM annihilations in the absence of a detectable spatially extended signal from the halo. We define two simple reference theories of DM with a thermal p-wave annihilation cross section and establish new limits on the combined particle and astrophysical parameter space of these models, demonstrating that Fermi Large Area Telescope is currently sensitive to thermal p-wave DM over a wide range of possible scenarios for the DM distribution in the GC.

  8. Significant gamma-ray lines from dark matter annihilation

    Energy Technology Data Exchange (ETDEWEB)

    Duerr, Michael [DESY, Notkestrasse 85, 22607 Hamburg (Germany); Fileviez Perez, Pavel; Smirnov, Juri [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, 69117 Heidelberg (Germany)

    2016-07-01

    Gamma-ray lines from dark matter annihilation are commonly seen as a ''smoking gun'' for the particle nature of dark matter. However, in many dark matter models the continuum background from tree-level annihilations makes such a line invisible. I present two simple extensions of the Standard Model where the continuum contributions are suppressed and the gamma-ray lines are easily visible over the continuum background.

  9. Breit-Wigner Enhancement of Dark Matter Annihilation

    Energy Technology Data Exchange (ETDEWEB)

    Ibe, Masahiro; /SLAC; Murayama, Hitoshi; /Tokyo U., IPMU /UC, Berkeley /LBL, Berkeley; Yanagida, T.T.; /Tokyo U. /Tokyo U., IPMU

    2009-06-19

    We point out that annihilation of dark matter in the galactic halo can be enhanced relative to that in the early universe due to a Breit-Wigner tail, if the dark matter annihilates through a pole just below the threshold. This provides a new explanation to the 'boost factor' which is suggested by the recent data of the PAMELA, ATIC and PPB-BETS cosmic-ray experiments.

  10. Polymerization of epoxy resins studied by positron annihilation

    International Nuclear Information System (INIS)

    Suzuki, T.; Hayashi, T.; Ito, Y.

    1999-01-01

    The polymerization process of epoxy resins (bisphenol-A dicyanate) was studied using positron-annihilation spectroscopy. The polymerization from monomer to polymer through a polymerization reaction was followed by positron-annihilation lifetime spectroscopy measurements. Resins kept at curing temperatures (120, 150 and 200 o C) changed form from of powder to a solid through a liquid. The size of the intermolecular spaces of the solid samples increased along with the progress of polymerization. (author)

  11. Fusion Reactions and Matter-Antimatter Annihilation for Space Propulsion

    Science.gov (United States)

    2005-07-13

    FUSION REACTIONS AND MATTER- ANTIMATTER ANNIHILATION FOR SPACE PROPULSION Claude DEUTSCH LPGP (UMR-CNRS 8578), Bât. 210, UPS, 91405 Orsay...REPORT TYPE N/A 3. DATES COVERED - 4. TITLE AND SUBTITLE šFusion Reactions And Matter- Antimatter Annihilation For Space Propulsion 5a...which is possible with successful MCF or ICF. Appropriate vessel designs will be presented for fusion as well as for antimatter propulsion. In

  12. The Characterization of the Gamma-Ray Signal from the Central Milky Way: A Compelling Case for Annihilating Dark Matter

    Energy Technology Data Exchange (ETDEWEB)

    Daylan, Tansu [Harvard Univ., Cambridge, MA (United States); Finkbeiner, Douglas P. [Harvard-Smithsonian Center, Cambridge, MA (United States); Hooper, Dan [Fermi National Accelerator Laboratory (FNAL), Batavia, IL (United States); Linden, Tim [Univ. of Illinois at Chicago, Chicago, IL (United States); Portillo, Stephen K. N. [Harvard-Smithsonian Center, Cambridge, MA (United States); Rodd, Nicholas L. [Massachusetts Institute of Technology, Boston, MA (United States); Slatyer, Tracy R. [Institute for Advanced Study, Princeton, NJ (United States)

    2014-02-26

    Past studies have identified a spatially extended excess of ~1-3 GeV gamma rays from the region surrounding the Galactic Center, consistent with the emission expected from annihilating dark matter. We revisit and scrutinize this signal with the intention of further constraining its characteristics and origin. By applying cuts to the Fermi event parameter CTBCORE, we suppress the tails of the point spread function and generate high resolution gamma-ray maps, enabling us to more easily separate the various gamma-ray components. Within these maps, we find the GeV excess to be robust and highly statistically significant, with a spectrum, angular distribution, and overall normalization that is in good agreement with that predicted by simple annihilating dark matter models. For example, the signal is very well fit by a 31-40 GeV dark matter particle annihilating to b quarks with an annihilation cross section of sigma v = (1.4-2.0) x 10^-26 cm^3/s (normalized to a local dark matter density of 0.3 GeV/cm^3). Furthermore, we confirm that the angular distribution of the excess is approximately spherically symmetric and centered around the dynamical center of the Milky Way (within ~0.05 degrees of Sgr A*), showing no sign of elongation along or perpendicular to the Galactic Plane. The signal is observed to extend to at least 10 degrees from the Galactic Center, disfavoring the possibility that this emission originates from millisecond pulsars.

  13. Structure formation constraints on Sommerfeld-enhanced dark matter annihilation

    International Nuclear Information System (INIS)

    Armendariz-Picon, Cristian; Neelakanta, Jayanth T.

    2012-01-01

    We study the growth of cosmic structure in a ΛCDM universe under the assumption that dark matter self-annihilates with an averaged cross section times relative velocity that grows with the scale factor, an increase known as Sommerfeld-enhancement. Such an evolution is expected in models in which a light force carrier in the dark sector enhances the annihilation cross section of dark matter particles, and has been invoked, for instance, to explain anomalies in cosmic ray spectra reported in the past. In order to make our results as general as possible, we assume that dark matter annihilates into a relativistic species that only interacts gravitationally with the standard model. This assumption also allows us to test whether the additional relativistic species mildly favored by cosmic-microwave background data could originate from dark matter annihilation. We do not find evidence for Sommerfeld-enhanced dark matter annihilation and derive the corresponding upper limits on the annihilation cross-section

  14. Positron Transport and Annihilation in the Galactic Bulge

    Directory of Open Access Journals (Sweden)

    Fiona Helen Panther

    2018-03-01

    Full Text Available The annihilation of positrons in the Milky Way Galaxy has been observed for ∼50 years; however, the production sites of these positrons remains hard to identify. The observed morphology of positron annihilation gamma-rays provides information on the annihilation sites of these Galactic positrons. It is understood that the positrons responsible for the annihilation signal originate at MeV energies. The majority of sources of MeV positrons occupy the star-forming thin disk of the Milky Way. If positrons propagate far from their sources, we must develop accurate models of positron propagation through all interstellar medium (ISM phases in order to reveal the currently uncertain origin of these Galactic positrons. On the other hand, if positrons annihilate close to their sources, an alternative source of MeV positrons with a distribution that matches the annihilation morphology must be identified. In this work, I discuss the various models that have been developed to understand the origin of the 511 keV line from the direction of the Galactic bulge, and the propagation of positrons in the ISM.

  15. Cosmic gamma-ray background from dark matter annihilation

    International Nuclear Information System (INIS)

    Ando, Shin'ichiro

    2007-01-01

    High-energy photons from pair annihilation of dark matter particles contribute to the cosmic gamma-ray background (CGB) observed in a wide energy range. The precise shape of the energy spectrum of CGB depends on the nature of dark matter particles. In order to discriminate between the signals from dark matter annihilation and other astrophysical sources, however, the information from the energy spectrum of CGB may not be sufficient. We show that dark matter annihilation not only contributes to the mean CGB intensity, but also produces a characteristic anisotropy, which provides a powerful tool for testing the origins of the observed CGB. We show that the expected sensitivity of future gamma-ray detectors such as GLAST should allow us to measure the angular power spectrum of CGB anisotropy, if dark matter particles are supersymmetric neutralinos and they account for most of the observed mean intensity. As the intensity of photons from annihilation is proportional to the density squared, we show that the predicted shape of the angular power spectrum of gamma rays from dark matter annihilation is different from that due to other astrophysical sources such as blazars, whose intensity is linearly proportional to density. Therefore, the angular power spectrum of the CGB provides a 'smoking-gun' signature of gamma rays from dark matter annihilation

  16. Efficient Homodifunctional Bimolecular Ring-Closure Method for Cyclic Polymers by Combining RAFT and Self-Accelerating Click Reaction.

    Science.gov (United States)

    Qu, Lin; Sun, Peng; Wu, Ying; Zhang, Ke; Liu, Zhengping

    2017-08-01

    An efficient metal-free homodifunctional bimolecular ring-closure method is developed for the formation of cyclic polymers by combining reversible addition-fragmentation chain transfer (RAFT) polymerization and self-accelerating click reaction. In this approach, α,ω-homodifunctional linear polymers with azide terminals are prepared by RAFT polymerization and postmodification of polymer chain end groups. By virtue of sym-dibenzo-1,5-cyclooctadiene-3,7-diyne (DBA) as small linkers, well-defined cyclic polymers are then prepared using the self-accelerating double strain-promoted azide-alkyne click (DSPAAC) reaction to ring-close the azide end-functionalized homodifunctional linear polymer precursors. Due to the self-accelerating property of DSPAAC ring-closing reaction, this novel method eliminates the requirement of equimolar amounts of telechelic polymers and small linkers in traditional bimolecular ring-closure methods. It facilitates this method to efficiently and conveniently produce varied pure cyclic polymers by employing an excess molar amount of DBA small linkers. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  17. Folding topology of a bimolecular DNA quadruplex containing a stable mini-hairpin motif within the diagonal loop.

    Science.gov (United States)

    Balkwill, Graham D; Garner, Thomas P; Williams, Huw E L; Searle, Mark S

    2009-02-06

    We describe the NMR structural characterisation of a bimolecular anti-parallel DNA quadruplex d(G(3)ACGTAGTG(3))(2) containing an autonomously stable mini-hairpin motif inserted within the diagonal loop. A folding topology is identified that is different from that observed for the analogous d(G(3)T(4)G(3))(2) dimer with the two structures differing in the relative orientation of the diagonal loops. This appears to reflect specific base stacking interactions at the quadruplex-duplex interface that are not present in the structure with the T(4)-loop sequence. A truncated version of the bimolecular quadruplex d(G(2)ACGTAGTG(2))(2), with only two core G-tetrads, is less stable and forms a heterogeneous mixture of three 2-fold symmetric quadruplexes with different loop arrangements. We demonstrate that the nature of the loop sequence, its ability to form autonomously stable structure, the relative stabilities of the hairpin loop and core quadruplex, and the ability to form favourable stacking interactions between these two motifs are important factors in controlling DNA G-quadruplex topology.

  18. Antimatter annihilation detection with AEgIS

    CERN Document Server

    Gligorova, Angela

    2015-01-01

    AE ̄ gIS (Antimatter Experiment: Gravity, Interferometry, Spectroscopy) is an antimatter exper- iment based at CERN, whose primary goal is to carry out the first direct measurement of the Earth’s gravitational acceleration on antimatter. A precise measurement of antimatter gravity would be the first precision test of the Weak Equivalence Principle for antimatter. The principle of the experiment is based on the formation of antihydrogen through a charge exchange reaction between laser excited (Rydberg) positronium and ultra-cold antiprotons. The antihydrogen atoms will be accelerated by an inhomogeneous electric field (Stark acceleration) to form a pulsed cold beam. The free fall of the antihydrogen due to Earth’s gravity will be measured using a moiré de- flectometer and a hybrid position detector. This detector is foreseen to consist of an active silicon part, where the annihilation of antihydrogen takes place, followed by an emulsion part coupled to a fiber time-of-flight detector. This overview prese...

  19. Positron annihilation lifetime spectroscopy of macromolecules

    International Nuclear Information System (INIS)

    Simon, G.

    1996-01-01

    Positron annihilation lifetime spectroscopy (PALS) is a technique which makes use of the anti- particle of the electron, the positron (e + ), first predicted by Dirac in 1931. This talk will concentrate on the use of PALS as a technique in characterising macromolecules. PALS has been used by various groups to evaluate many properties that one associates with free volume such as physical ageing, gas permeability, the glass transition, uptake of a solvent, crystallinity, crosslinking, molecular mobility. One area of much interest has been the use of this technique in looking at miscibility of polymer blends. In miscible blends, the interactions of the different polymers may be expected to lead to a negative free volume of mixing because of the strong attraction between the different chains. This may influence the free volume properties. Conversely, if a material is partially miscible or totally immiscible, this should influence both the size and total content of free volume. This should be related to other properties such as mechanical properties and molecular mobility, such as measured by dielectric relaxation spectroscopy. Variations on this involve copolymerization of crosslinked materials or linear thermoplastics (the ultimate 'molecular' miscibility) and this will also be discussed. Multiphase systems such as water uptake in polymers can vary polymer properties by filling molecular voids, as well as disturbing chain conformations and, in the case of polar polymers, associating with the polymer chains. The effect of polymer molecular structure on free volume - particularly in rigid polymer chains such as substituted poly(phenylenes) and liquid crystalline polymers will also be presented. Indeed, the unusual packing which arises from such anisotropic molecules leads to unusual behaviours both of the homolpolymers and subsequent liquid crystal polymer - liquid crystal polymer blends

  20. On fascination and fear of annihilation.

    Science.gov (United States)

    Thys, Michel

    2017-06-01

    In this paper fascination phenomenologically is described as a state of radically being captured by an imposing object. What is left of the impoverished and paralysed subject clings to the exclusive fascinating object. Fascination is the eye of the storm of extreme ambivalence towards an exclusive object: being the only remaining object it is necessary for living in an object world, but at the same time it is threatening to life by absorbing the subject totally. So the subject is sucked in by a yet frightening object. From a metapsychological point of view fascination is understood as the congealed result of excessive projective identification and a strong confusional state connected with it: the subject empties itself so much in the object that it comes to stand for the subject. The fascinating object embodies in a condensed way - as a special form of a bizarre object - split off unconscious threatening material. So fascination is linked to the Kleinian theory of anxiety. Two clinical vignettes illustrate how states of fascination can be understood as an ultimate defence against unconscious menacing material welling up. The hypothesis is developed that fascination points to a revelation of fundamental psychic truth that promptly cramps the subject because the reintegration of it is felt as annihilating. In the vignettes this takes the form of a 'transformation in hallucinosis'. Fascination is at the same time 'the moment of truth' and possibly a serious obstruction of the analytic process. This unconscious truth seems to concern primitive 'superego violence'. The challenge consists in thawing the frozen fascinating object by linking it to other material. Copyright © 2016 Institute of Psychoanalysis.

  1. Substructure boosts to dark matter annihilation from Sommerfeld enhancement

    International Nuclear Information System (INIS)

    Bovy, Jo

    2009-01-01

    The recently introduced Sommerfeld enhancement of the dark matter annihilation cross section has important implications for the detection of dark matter annihilation in subhalos in the Galactic halo. In addition to the boost to the dark matter annihilation cross section from the high densities of these subhalos with respect to the main halo, an additional boost caused by the Sommerfeld enhancement results from the fact that they are kinematically colder than the Galactic halo. If we further believe the generic prediction of the cold dark matter paradigm that in each subhalo there is an abundance of substructure which is approximately self-similar to that of the Galactic halo, then I show that additional boosts coming from the density enhancements of these small substructures and their small velocity dispersions enhance the dark matter annihilation cross section even further. I find that very large boost factors (10 5 to 10 9 ) are obtained in a large class of models. The implications of these boost factors for the detection of dark matter annihilation from dwarf spheroidal galaxies in the Galactic halo are such that, generically, they outshine the background gamma-ray flux and are detectable by the Fermi Gamma-ray Space Telescope.

  2. The influence of antioxidant on positron annihilation in polypropylene

    International Nuclear Information System (INIS)

    Djourelov, N.; He, C.; Suzuki, T.; Ito, Y; Kondo, K.; Ito, Y.; Shantarovich, V.P.

    2003-01-01

    The purpose of this report is to check the influence of the carbonyl groups (CG), created by oxygen naturally dissolved in a polymer matrix and by the source irradiation, on annihilation characteristics of free positrons using the positron annihilation lifetime spectroscopy (PALS) and coincidence Doppler-broadening spectroscopy (CDBS). Positron annihilation in a pure polypropylene (PP) and in an antioxidant-containing polypropylene (PPA) sample at room and low temperatures has been studied by CDBS. PALS has been used as an o-Ps (orth-positronium) formation monitor. The momentum density distributions of electrons obtained by CDBS at the beginning of measurements have been compared to that at the o-Ps intensity saturation level. It has been shown that the initial concentration of carbonyl groups in a PP sample is high, while for an antioxidant-containing sample, PPA, carbonyl groups are not detected by CDBS. CDBS spectra for a PP can be explained by annihilation of free positrons with the oxygen contained in the carbonyl groups. For a PPA sample, no significant contribution of annihilation with oxygen core electrons can be concluded. (Y. Kazumata)

  3. The Isotropic Radio Background and Annihilating Dark Matter

    Energy Technology Data Exchange (ETDEWEB)

    Hooper, Dan [Fermi National Accelerator Laboratory (FNAL), Batavia, IL (United States); Belikov, Alexander V. [Institut d' Astrophysique (France); Jeltema, Tesla E. [Univ. of California, Santa Cruz, CA (United States); Linden, Tim [Univ. of California, Santa Cruz, CA (United States); Profumo, Stefano [Univ. of California, Santa Cruz, CA (United States); Slatyer, Tracy R. [Princeton Univ., Princeton, NJ (United States)

    2012-11-01

    Observations by ARCADE-2 and other telescopes sensitive to low frequency radiation have revealed the presence of an isotropic radio background with a hard spectral index. The intensity of this observed background is found to exceed the flux predicted from astrophysical sources by a factor of approximately 5-6. In this article, we consider the possibility that annihilating dark matter particles provide the primary contribution to the observed isotropic radio background through the emission of synchrotron radiation from electron and positron annihilation products. For reasonable estimates of the magnetic fields present in clusters and galaxies, we find that dark matter could potentially account for the observed radio excess, but only if it annihilates mostly to electrons and/or muons, and only if it possesses a mass in the range of approximately 5-50 GeV. For such models, the annihilation cross section required to normalize the synchrotron signal to the observed excess is sigma v ~ (0.4-30) x 10^-26 cm^3/s, similar to the value predicted for a simple thermal relic (sigma v ~ 3 x 10^-26 cm^3/s). We find that in any scenario in which dark matter annihilations are responsible for the observed excess radio emission, a significant fraction of the isotropic gamma ray background observed by Fermi must result from dark matter as well.

  4. THE EFFECTS OF DARK MATTER ANNIHILATION ON COSMIC REIONIZATION

    Energy Technology Data Exchange (ETDEWEB)

    Kaurov, Alexander A.; Hooper, Dan; Gnedin, Nickolay Y., E-mail: kaurov@uchicago.edu [Department of Astronomy and Astrophysics, The University of Chicago, Chicago, IL 60637 (United States)

    2016-12-20

    We revisit the possibility of constraining the properties of dark matter (DM) by studying the epoch of cosmic reionization. Previous studies have shown that DM annihilation was unlikely to have provided a large fraction of the photons which ionized the universe, but instead played a subdominant role relative to stars and quasars. The DM might, however, have begun to efficiently annihilate with the formation of primordial microhalos at z  ∼ 100–200, much earlier than the formation of the first stars. Therefore, if DM annihilation ionized the universe at even the percent level over the interval z  ∼ 20–100, it could leave a significant imprint on the global optical depth, τ . Moreover, we show that cosmic microwave background polarization data and future 21 cm measurements will enable us to more directly probe the DM contribution to the optical depth. In order to compute the annihilation rate throughout the epoch of reionization, we adopt the latest results from structure formation studies and explore the impact of various free parameters on our results. We show that future measurements could make it possible to place constraints on the DM’s annihilation cross-sections, which are at a level comparable to those obtained from the observations of dwarf galaxies, cosmic-ray measurements, and studies of recombination.

  5. Dark matter annihilation in the circumgalactic medium at high redshifts

    Science.gov (United States)

    Schön, S.; Mack, K. J.; Wyithe, J. S. B.

    2018-03-01

    Annihilating dark matter (DM) models offer promising avenues for future DM detection, in particular via modification of astrophysical signals. However, when modelling such potential signals at high redshift, the emergence of both DM and baryonic structure, as well as the complexities of the energy transfer process, needs to be taken into account. In the following paper, we present a detailed energy deposition code and use this to examine the energy transfer efficiency of annihilating DM at high redshift, including the effects on baryonic structure. We employ the PYTHIA code to model neutralino-like DM candidates and their subsequent annihilation products for a range of masses and annihilation channels. We also compare different density profiles and mass-concentration relations for 105-107 M⊙ haloes at redshifts 20 and 40. For these DM halo and particle models, we show radially dependent ionization and heating curves and compare the deposited energy to the haloes' gravitational binding energy. We use the `filtered' annihilation spectra escaping the halo to calculate the heating of the circumgalactic medium and show that the mass of the minimal star-forming object is increased by a factor of 2-3 at redshift 20 and 4-5 at redshift 40 for some DM models.

  6. Charge effect on the diffusion coefficient and the bimolecular reaction rate of diiodide anion radical in room temperature ionic liquids.

    Science.gov (United States)

    Nishiyama, Yoshio; Terazima, Masahide; Kimura, Yoshifumi

    2009-04-16

    The diffusion coefficients of diiodide anion radical, I(2)(-), in room temperature ionic liquids (RTILs) were determined by the transient grating (TG) method using the photochemical reaction of iodide. The diffusion coefficients we obtained were larger in RTILs than the theoretical predictions by the Stokes-Einstein relation, whereas both values are similar in conventional solvents. By comparison with the diffusion coefficients of neutral molecules, it was suggested that the Coulomb interaction between I(2)(-) and constituent ions of RTILs strongly affects the diffusion coefficients. The bimolecular reaction rates between I(2)(-) were calculated by the Debye-Smoluchowski equation using the experimentally determined diffusion coefficients. These calculated reaction rate were much smaller than the experimentally determined rates (Takahashi, K.; et al. J. Phys. Chem. B 2007, 111, 4807), indicating the charge screening effect of RTILs.

  7. Kinetics and Mechanism of the CIO + CIO Reaction: Pressure and Temperature Dependences of the Bimolecular and Termolecular Channels andThermal Decomposition of Chlorine Peroxide, CIOOCI

    Science.gov (United States)

    Nickolaisen, Scott L.; Friedl, Randall R.; Sander, Stanley P.

    1993-01-01

    The kinetics and mechanism of the CIO + CIO reaction and the thermal decomposition of CIOOCI were studied using the flash photolysis/long path ultraviolet absorption technique. Pressure and temperature dependences were determined for the rate coefficients for the bimolecular and termolecular reaction channels, and for the thermal decompositon of CIOOCI.

  8. The dating game at dimension zero: creation and annihilation of phase singularities in optical random waves

    NARCIS (Netherlands)

    De Angelis, L.; Alpeggiani, F.; Di Falco, Andrea; Kuipers, L.

    2017-01-01

    Phase singularities can be created and annihilated, but always in pairs. With optical near-field measurements, we track singularities in random waves as a function of wavelength, and discover correlations between creation and annihilation events.

  9. Models of pair annihilation in 1E 1740.7-2942 and the HEAO 1 A-4 annihilation source

    Science.gov (United States)

    Maciolek-Niedzwiecki, Andrzej; Zdziarski, Andrzej

    1994-01-01

    We study possible models of two Galactic sources of transient pair annihilation radiation, 1E 1740.7-2942 and a source observed by High Energy Astronomy Observatory (HEAO) 1 A-4. We fit the observed spectral features by thermal annihilation spectra and find that the redshifts obtained by us are much larger than those obtained from fitting Caussian lines centered on 511 keV. This effect, which is due to the net blueshift (with respect to 511 keV) of the annihilation spectrum due to the thermal energies of pairs, puts strong constraints on models of sources. We consider those constraints first without considering the mechanism of positron production. From the shape of the observed spectra, we are able to rule out both spherical clouds and layers above cold matter as possible source geometries. The observed spectra are compatible with two source geometries: (1) a nearly face-on disk in the Kerr metric and (2) a jet close to a black hole. We consider, then, the origin of the pairs. Theories of both thermal and nonthermal pair equilibria predict that photon-pair production is unable to produce annihilation features that contain as much as half of the bolometric luminosity, which is observed. A possible solution to this problem is obscuration of a nonthermal source (in which pairs are produced by photon-photon collisions) and an outflow of pairs to an unobscured region. This makes annihilation in a jet the most likely model of the considered sources.

  10. The Distribution and Annihilation of Dark Matter Around Black Holes

    Science.gov (United States)

    Schnittman, Jeremy D.

    2015-01-01

    We use a Monte Carlo code to calculate the geodesic orbits of test particles around Kerr black holes, generating a distribution function of both bound and unbound populations of dark matter (DM) particles. From this distribution function, we calculate annihilation rates and observable gamma-ray spectra for a few simple DM models. The features of these spectra are sensitive to the black hole spin, observer inclination, and detailed properties of the DM annihilation cross-section and density profile. Confirming earlier analytic work, we find that for rapidly spinning black holes, the collisional Penrose process can reach efficiencies exceeding 600%, leading to a high-energy tail in the annihilation spectrum. The high particle density and large proper volume of the region immediately surrounding the horizon ensures that the observed flux from these extreme events is non-negligible.

  11. Internal-fusion diagrams for p-barp annihilation

    Energy Technology Data Exchange (ETDEWEB)

    Genz, H.; Tatur, S.

    1984-07-01

    We investigate p-barp annihilation into B-barB' (where B and B' represent baryons) via q-barq annihilation into Q-barQ (where q and Q represent quarks). Specifying the q-barq (or q-barQ) annihilation spin structure determines the ratios of all polarized amplitudes with B,B' from the 56 under SU(6). We propose to parametrize q-barq..-->..Q-barQ by intermediate gluon and meson states. The model with q-barq..-->..one gluon..-->..Q-barQ with Q = s is worked out in detail. With the exception of p-barp..-->..Sigma-bar/sup -/..sigma../sup asterisk+/+charge conjugate, it compares favorably with experiment.

  12. Notes on symmetric and exterior depth and annihilator numbers

    Directory of Open Access Journals (Sweden)

    Gesa Kampf

    2008-11-01

    Full Text Available We survey and compare invariants of modules over the polynomial ring and the exterior algebra. In our considerations, we focus on the depth. The exterior analogue of depth was first introduced by Aramova, Avramov and Herzog. We state similarities between the two notion of depth and exhibit their relation in the case of squarefree modules. Work of Conca, Herzog and Hibi and Trung, respectively, shows that annihilator numbers are a meaningful generalization of depth over the polynomial ring. We introduce and study annihilator numbers over the exterior algebra. Despite some minor differences in the definition, those invariants show common behavior. In both situations a positive linear combination of the annihilator numbers can be used to bound the symmetric and exterior graded Betti numbers, respectively, from above.

  13. Molecular model for annihilation rates in positron complexes

    International Nuclear Information System (INIS)

    Assafrao, Denise; Walters, H.R. James; Mohallem, Jose R.

    2008-01-01

    The molecular approach for positron interaction with atoms is developed further. Potential energy curves for positron motion are obtained. Two procedures accounting for the nonadiabatic effective positron mass are introduced for calculating annihilation rate constants. The first one takes the bound-state energy eigenvalue as an input parameter. The second is a self-contained and self-consistent procedure. The methods are tested with quite different states of the small complexes HPs, e + He (electronic triplet) and e + Be (electronic singlet and triplet). For states yielding the positronium cluster, the annihilation rates are quite stable, irrespective of the accuracy in binding energies. For the e + Be states, annihilation rates are larger and more consistent with qualitative predictions than previously reported ones

  14. Positron annihilation in germanium in thermal equilibrium at high temperature

    Energy Technology Data Exchange (ETDEWEB)

    Uedono, Akira; Moriya, Tsuyoshi; Komuro, Naoyuki; Tanigawa, Shoichiro [Tsukuba Univ., Ibaraki (Japan). Inst. of Materials Science; Kawano, Takao; Ikari, Atsushi

    1996-09-01

    Annihilation characteristics of positrons in Ge in thermal equilibrium at high temperature were studied using a monoenergetic positron beam. Precise measurements of Doppler broadening profiles of annihilation radiation were performed in the temperature range between 300 K and 1211 K. The line shape parameters of Doppler broadening profiles were found to be almost constant at 300-600 K. The changes in these parameters were observed to start above 600 K. This was attributed to both the decrease in the fraction of positrons annihilating with core electrons and the lowering of the crystal symmetry around the region detected by positron-electron pairs. This suggests that behaviors of positrons are dominated by some form of positron-lattice coupling in Ge at high temperatures. The temperature dependence of the diffusion length of positrons was also discussed. (author)

  15. Molecular model for annihilation rates in positron complexes

    Energy Technology Data Exchange (ETDEWEB)

    Assafrao, Denise [Laboratorio de Atomos e Moleculas Especiais, Departamento de Fisica, ICEx, Universidade Federal de Minas Gerais, P.O. Box 702, 30123-970 Belo Horizonte, MG (Brazil); Department of Applied Mathematics and Theoretical Physics, Queen' s University of Belfast, Belfast BT7 1NN, Northern Ireland (United Kingdom); Walters, H.R. James [Department of Applied Mathematics and Theoretical Physics, Queen' s University of Belfast, Belfast BT7 1NN, Northern Ireland (United Kingdom); Mohallem, Jose R. [Laboratorio de Atomos e Moleculas Especiais, Departamento de Fisica, ICEx, Universidade Federal de Minas Gerais, P.O. Box 702, 30123-970 Belo Horizonte, MG (Brazil); Department of Applied Mathematics and Theoretical Physics, Queen' s University of Belfast, Belfast BT7 1NN, Northern Ireland (United Kingdom)], E-mail: rachid@fisica.ufmg.br

    2008-02-15

    The molecular approach for positron interaction with atoms is developed further. Potential energy curves for positron motion are obtained. Two procedures accounting for the nonadiabatic effective positron mass are introduced for calculating annihilation rate constants. The first one takes the bound-state energy eigenvalue as an input parameter. The second is a self-contained and self-consistent procedure. The methods are tested with quite different states of the small complexes HPs, e{sup +}He (electronic triplet) and e{sup +}Be (electronic singlet and triplet). For states yielding the positronium cluster, the annihilation rates are quite stable, irrespective of the accuracy in binding energies. For the e{sup +}Be states, annihilation rates are larger and more consistent with qualitative predictions than previously reported ones.

  16. Simulation of structure and annihilation of screw dislocation dipoles

    DEFF Research Database (Denmark)

    Rasmussen, Torben; Vegge, Tejs; Leffers, Torben

    2000-01-01

    Large scale atomistic simulations are used to investigate the properties of screw dislocation dipoles in copper. Spontaneous annihilation is observed for dipole heights less than 1 nm. Equilibrated dipoles of heights larger than 1 nm adopt a skew configuration due to the elastic anisotropy of Cu....... The equilibrium splitting width of the screw dislocations decreases with decreasing dipole height, as expected from elasticity theory. The energy barriers, and corresponding transition states for annihilation of stable dipoles are determined for straight and for flexible dislocations for dipole heights up to 5.......2 nm. In both cases the annihilation is initiated by cross-slip of one of the dislocations. For straight dislocations the activation energy shows a linear dependence on the inverse dipole height, and for flexible dislocations the dependence is roughly linear for the dipoles investigated....

  17. Singlet-triplet annihilation in single LHCII complexes.

    Science.gov (United States)

    Gruber, J Michael; Chmeliov, Jevgenij; Krüger, Tjaart P J; Valkunas, Leonas; van Grondelle, Rienk

    2015-08-14

    In light harvesting complex II (LHCII) of higher plants and green algae, carotenoids (Cars) have an important function to quench chlorophyll (Chl) triplet states and therefore avoid the production of harmful singlet oxygen. The resulting Car triplet states lead to a non-linear self-quenching mechanism called singlet-triplet (S-T) annihilation that strongly depends on the excitation density. In this work we investigated the fluorescence decay kinetics of single immobilized LHCIIs at room temperature and found a two-exponential decay with a slow (3.5 ns) and a fast (35 ps) component. The relative amplitude fraction of the fast component increases with increasing excitation intensity, and the resulting decrease in the fluorescence quantum yield suggests annihilation effects. Modulation of the excitation pattern by means of an acousto-optic modulator (AOM) furthermore allowed us to resolve the time-dependent accumulation and decay rate (∼7 μs) of the quenching species. Inspired by singlet-singlet (S-S) annihilation studies, we developed a stochastic model and then successfully applied it to describe and explain all the experimentally observed steady-state and time-dependent kinetics. That allowed us to distinctively identify the quenching mechanism as S-T annihilation. Quantitative fitting resulted in a conclusive set of parameters validating our interpretation of the experimental results. The obtained stochastic model can be generalized to describe S-T annihilation in small molecular aggregates where the equilibration time of excitations is much faster than the annihilation-free singlet excited state lifetime.

  18. Relativistic hydrodynamics, heavy ion reactions and antiproton annihilation

    International Nuclear Information System (INIS)

    Strottman, D.

    1985-01-01

    The application of relativistic hydrodynamics to relativistic heavy ions and antiproton annihilation is summarized. Conditions for validity of hydrodynamics are presented. Theoretical results for inclusive particle spectra, pion production and flow analysis are given for medium energy heavy ions. The two-fluid model is introduced and results presented for reactions from 800 MeV per nucleon to 15 GeV on 15 GeV per nucleon. Temperatures and densities attained in antiproton annihilation are given. Finally, signals which might indicate the presence of a quark-gluon plasma are briefly surveyed

  19. Investigation of highly activated materials by conventional positron annihilation spectroscopy

    International Nuclear Information System (INIS)

    Sabelova, V.; Petriska, M.; Slugen, V.; Krsjak, V.

    2013-01-01

    Positron annihilation process is helpful tool for material microstructure study. Many useful methods for detecting vacancies and their clusters in various alloys use its principle. Experimental procedure of positron source preparation (radioactive 22 Na) for these methods is difficult task. The unusual small sample dimensions of studied irradiated Eurofer 97 alloy form difficult conditions for its manufacturing. The unique sodium positron source proper preparation is confirmed by positron annihilation lifetime spectroscopy (PALS) and coincidence Doppler broadening spectroscopy (CDBS) in Paul Scherrer Institute in Switzerland. (authors)

  20. Application of positron annihilation technique to reverse osmosis membrane materials

    International Nuclear Information System (INIS)

    Shimazu, A.; Ikeda, K.; Miyazaki, T.; Ito, Y.

    2000-01-01

    Positron annihilation lifetime spectroscopy has been adopted as a new approach for studying vacancies of reverse osmosis membrane materials composed of cellulose acetate films and aromatic polyamide resins. The intensity of the ortho-positronium (o-Ps) lifetime increased with the amount of vacancies determined using N 2 isotherm at -195 deg. C. Changes of vacancy profiles induced by heat treatment in the cellulose acetate films were detected using o-Ps. It was found that the positron annihilation technique is applicable to the study of vacancy profiles associated with salt selectivity in typical reverse osmosis membranes.

  1. Annihilation physics of exotic galactic dark matter particles

    Science.gov (United States)

    Stecker, F. W.

    1990-01-01

    Various theoretical arguments make exotic heavy neutral weakly interacting fermions, particularly those predicted by supersymmetry theory, attractive candidates for making up the large amount of unseen gravitating mass in galactic halos. Such particles can annihilate with each other, producing secondary particles of cosmic-ray energies, among which are antiprotons, positrons, neutrinos, and gamma-rays. Spectra and fluxes of these annihilation products can be calculated, partly by making use of positron electron collider data and quantum chromodynamic models of particle production derived therefrom. These spectra may provide detectable signatures of exotic particle remnants of the big bang.

  2. Computer Simulation of Electron Positron Annihilation Processes

    Energy Technology Data Exchange (ETDEWEB)

    Chen, y

    2003-10-02

    With the launching of the Next Linear Collider coming closer and closer, there is a pressing need for physicists to develop a fully-integrated computer simulation of e{sup +}e{sup -} annihilation process at center-of-mass energy of 1TeV. A simulation program acts as the template for future experiments. Either new physics will be discovered, or current theoretical uncertainties will shrink due to more accurate higher-order radiative correction calculations. The existence of an efficient and accurate simulation will help us understand the new data and validate (or veto) some of the theoretical models developed to explain new physics. It should handle well interfaces between different sectors of physics, e.g., interactions happening at parton levels well above the QCD scale which are described by perturbative QCD, and interactions happening at much lower energy scale, which combine partons into hadrons. Also it should achieve competitive speed in real time when the complexity of the simulation increases. This thesis contributes some tools that will be useful for the development of such simulation programs. We begin our study by the development of a new Monte Carlo algorithm intended to perform efficiently in selecting weight-1 events when multiple parameter dimensions are strongly correlated. The algorithm first seeks to model the peaks of the distribution by features, adapting these features to the function using the EM algorithm. The representation of the distribution provided by these features is then improved using the VEGAS algorithm for the Monte Carlo integration. The two strategies mesh neatly into an effective multi-channel adaptive representation. We then present a new algorithm for the simulation of parton shower processes in high energy QCD. We want to find an algorithm which is free of negative weights, produces its output as a set of exclusive events, and whose total rate exactly matches the full Feynman amplitude calculation. Our strategy is to create

  3. Effect of Voids on Angular Correlation of Positron Annihilation Photons in Molybdenum

    DEFF Research Database (Denmark)

    Mogensen, O. E.; Petersen, K.; Cotterill, R. M. J.

    1972-01-01

    POSITRON annihilation investigations of defects in crystals have shown that for sufficiently high defect concentrations (typically above about 10−6) all positrons become trapped in the defects before annihilation, thus changing the characteristics of the annihilation process. For example, trapping...... be disturbed either in a random fashion or arranged in a macro lattice7....

  4. Origin and annihilation physics of positrons in the Galaxy

    International Nuclear Information System (INIS)

    Alexis, Anthony

    2014-01-01

    A gamma radiation at 511 keV is observed since the early 1970's toward the Galactic bulge region. This emission is the signature of a large number of electron-positron annihilations, the positron being the electron's antiparticle. Unfortunately, the origin of the positrons responsible for this emission is still a mystery. Many positron-source candidates have been suggested but none of them can account for the galactic annihilation emission. The spatial distribution of this emission is indeed very atypical. Since 2002, the SPI spectrometer onboard the INTEGRAL space laboratory revealed an emission strongly concentrated toward the galactic bulge and a weaker emission from the galactic disk. This morphology is unusual because it does not correspond to any of the known galactic astrophysical-object or interstellar-matter distributions. The assumption that positrons annihilate close to their sources (i.e. the spatial distribution of the annihilation emission reflects the spatial distribution of the sources) has consequently been called into question. Recent studies suggest that positrons could propagate far away from their sources before annihilating. This physical aspect could be the key point to solve the riddle of the galactic positron origin. This thesis is devoted to the modelling of the propagation and annihilation of positrons in the Galaxy, in order to compare simulated spatial models of the annihilation emission with recent measurements provided by SPI/INTEGRAL. This method allows to put constraints on the origin of galactic positrons. We therefore developed a propagation Monte-Carlo code of positrons within the Galaxy in which we implemented all the theoretical and observational knowledge about positron physics (sources, transport modes, energy losses, annihilation modes) and the interstellar medium of our Galaxy (interstellar gas distributions, galactic magnetic fields, structures of the gaseous phases). Due to uncertainties in several physical parameters

  5. The influence of the quencher concentration on the rate of simple bimolecular reaction: molecular dynamics study. II.

    Science.gov (United States)

    Litniewski, Marek

    2006-03-21

    In this paper new results of the simulations [M. Litniewski, J. Chem. Phys. 123, 124506 (2005)] on the influence of the quencher concentration on the reaction A+B-->C+B for the identical soft sphere system are presented. The problem is generalized by considering also the case when the spheres are immersed in the Brownian medium. A significant difference between simple deterministic systems and the Brownian ones is found: the excess in the rate coefficient for the Brownian system is constant and positive, except for very short times. The reaction has been simulated for a very long time, but any tendency to decrease the excess has not been noted. It is also shown that the relative excess in the surviving probability is a universal quadratic function of the quencher concentration for the range of time much longer than the result from the previous simulations. A very strong correlation between the excess in the relative value of spatial correlations between the reagents and the excess in the rate coefficient is shown. It is also shown that the A-A and A-C interactions have some influence on the excess values. A simple model for this effect is presented.

  6. Annihilation limit of a visible-to-UV photon upconversion composition ascertained from transient absorption kinetics.

    Science.gov (United States)

    Deng, Fan; Blumhoff, Jörg; Castellano, Felix N

    2013-05-30

    Noncoherent sensitized green-to-near-visible upconversion has been achieved utilizing palladium(II) octaethylporphyrin (PdOEP) as the triplet sensitizer and anthracene as the energy acceptor/annihilator in vacuum degassed toluene. Selective 547 nm excitation of PdOEP with incident irradiance as low as 600 μW/cm(2) results in the observation of anthryl fluorescence at higher energy. Stern-Volmer analysis of the dynamic phosphorescence quenching of PdOEP by anthracene possesses an extremely large K(SV) of 810,000 M(-1), yielding a triplet-triplet energy transfer quenching constant of 3.3 × 10(9) M(-1) s(-1). Clear evidence for the subsequent triplet-triplet annihilation (TTA) of anthracene was afforded by numerous experiments, one of the most compelling was an excitation scan illustrating that the Q-band absorption features of PdOEP are solely responsible for sensitizing the anti-Stokes fluorescence. The upconverted emission intensity with respect to the excitation power was shown to vary between quadratic and linear using either coherent or noncoherent light sources, illustrating the expected kinetic limits for the light producing photochemistry under continuous wave illumination. Time-resolved experiments directly comparing the total integrated anthracene intensity/time fluorescence data produced through upconversion (λ(ex) = 547 nm, delayed signal) and with direct excitation (λ(ex) = 355 nm, prompt signal) under conditions where the laser pulse is completely absorbed by the sample reveal annihilation efficiencies of approximately 40%. Similarly, the delayed fluorescence kinetic analysis reported by Schmidt and co-workers (J. Phys. Chem. Lett. 2010, 1, 1795-1799) was used to reveal the maximum possible efficiency from a model red-to-yellow upconverting composition and this treatment was applied to the anthryl triplet absorption decay transients of anthracene measured for the PdOEP/anthracene composition at 430 nm. From this analysis approximately 50% of the

  7. Inverse Compton Gamma Rays from Dark Matter Annihilation in the ...

    Indian Academy of Sciences (India)

    didates for dark matter search due to their high mass-to-light (M/L) ratio. One of the most favored dark matter candidates is the lightest neutralino. (neutral χ particle) as predicted in the Minimal Supersymmetric Standard. Model (MSSM). In this study, we model the gamma ray emission from dark matter annihilation coming ...

  8. Precise tests of QCD in e+e- annihilation

    International Nuclear Information System (INIS)

    Burrows, P.N.

    1997-03-01

    A pedagogical review is given of precise tests of QCD in electron-positron annihilation. Emphasis is placed on measurements that have served to establish QCD as the correct theory of strong interactions, as well as measurements of the coupling parameter α s . An outlook is given for future important tests at a high-energy e + e - collider

  9. Study of wino pair production in e+e- annihilation

    International Nuclear Information System (INIS)

    Fukai, Tomoki; Kizukuri, Yoshiki; Oshimo, Noriyuki; Otake, Yoshie; Sugiyama, Naoshi

    1987-01-01

    We discuss wino pair production in e + e - annihilation and subsequent leptonic wino decay for various types of supersymmetric or supergravity models. Phenomenological predictions on this process depend considerably on a specific model. We analyze the energy distribution, forward-backward asymmetry and angular distribution of a charged lepton in the final state. (Author shortened by G.Q.)

  10. Monoenergetic neutrinos from dark matter annihilation: Issues of exposure

    Energy Technology Data Exchange (ETDEWEB)

    Kumar, Jason, E-mail: jkumar@hawaii.edu [Department of Physics and Astronomy, University of Hawai’i, Honolulu, HI 96822 (United States)

    2016-06-21

    We consider searches for dark matter annihilation in the Sun resulting in monoenergetic neutrinos, produced either directly or through the decay of stopped pions and kaons. We find that this strategy is very successful at increasing the signal-to-background ratio, but that current experiments may be signal limited. We discuss the exposures need to fully exploit this search strategy.

  11. Annihilation of the triplet excitons in the nanoporous glass matrices

    International Nuclear Information System (INIS)

    Afanasyev, D.A.; Ibrayev, N.Kh.; Saletsky, A.M.; Starokurov, Y.V.; Gun'ko, V.M.; Mikhalovsky, S.V.

    2013-01-01

    The spectra and kinetics of fluorescence decay of 1,2-benzanthracene (1,2-BA) molecular clusters adsorbed in nanoporous borosilicate glasses were investigated. It has been shown that the type of the decay kinetics of delayed fluorescence is determined by the annihilation of triplet excitons in crystalline and percolation clusters. The influence of an external magnetic field on the annihilation rate constant of triplet excitons in the adsorbed 1,2-BA molecules has been studied. The response of the molecular clusters to the magnetic field strongly depends on temperature, pore size and time scale of the observation. Clusters with the crystal structure dominate in the decay kinetics of triplet–triplet annihilation (TTA) and delayed fluorescence in the initial microsecond period of time after excitation. Amorphous clusters determine the form of decay kinetics of delayed fluorescence in the millisecond range. The increase in the pore size and concentration of the adsorbate lead to the dominance of crystalline components. The results presented here can be used to develop techniques for probing the structure of the adsorbed layer in nanoporous systems examining the effect of an external magnetic field on the annihilation delayed fluorescence (ADF) kinetics. Highlights: ► Molecular clusters of 1,2-benzanthracene adsorbed in nanoporous borosilicate glasses. ► Form of decay kinetics of delayed fluorescence. ► Magnetic field effects depend on temperature, pore size and observation time range. ► Clusters with crystal structure and amorphous clusters form in porous glasses

  12. Annihilation of Domain Walls in a Ferromagnetic Wire

    Science.gov (United States)

    Ghosh, Anirban; Huang, Kevin; Tchernyshyov, Oleg

    We study the annihilation of topological solitons in one of the simplest systems that support them: a one-dimensional ferromagnetic wire with an easy axis along its length. In the presence of energy dissipation due to viscous losses, two solitons (domain walls) on the wire, when released from afar, approach each other and eventually annihilate to create a uniformly magnetized state. Starting from a class of exact solutions for stationary two-domain-wall configurations in the absence of dissipation, we develop an effective theory that describes this annihilation in terms of four collective coordinates: a) the two zero modes corresponding to the location of the center and the average azimuthal angle of the full structure and b) their two conjugate momenta which describe the relative twist and the relative separation of the two domain walls respectively. Comparison with micromagnetic simulation on OOOMF confirms that this theory captures well the essential physics of the process. We believe this work will be a good starting point for studying the annihilation of more complicated topological solitons like vortices and skyrmions in ferromagnetic thin films. This work is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-FG02-08ER46544.

  13. Phase behaviour in confined geometry via positronium annihilation spectroscopy

    International Nuclear Information System (INIS)

    Fretwell, H.M.; Duffy, J.A.; Clarke, A.P.; Dugdale, S.B.; Alam, M.A.; Evans, R.

    1997-01-01

    Positronium annihilation spectroscopy has recently been successfully applied to the study of phase behaviour of fluids confined in nano-pores. In this paper we provide a brief survey of the new technique in mapping out the phase diagram in confinement and in elucidating some intricate phase behaviour. (author). 12 refs, 3 figs

  14. Significant Enhancement of Neutralino Dark Matter Annihilation from Electroweak Bremsstrahlung

    NARCIS (Netherlands)

    Bringmann, T.; Calore, F.

    2014-01-01

    ndirect searches for the cosmological dark matter have become ever more competitive during the past years. Here, we report the first full calculation of leading electroweak corrections to the annihilation rate of supersymmetric neutralino dark matter. We find that these corrections can be huge,

  15. Production of new particles in electron-positron annihilation

    International Nuclear Information System (INIS)

    Gilman, F.J.

    1977-02-01

    A number of areas are reviewed where there is important progress in the production of new particles in electron--positron annihilation, but of a more detailed quantitative nature. Charmonium states, charmed mesons, and evidence for a charged heavy lepton are covered. 50 references

  16. Chemical application of positron annihilation through triple coincidence measurement

    International Nuclear Information System (INIS)

    Yegnasubramanian, S.; Gangadharan, S.

    1982-01-01

    This report summarises the work on the application of triple coincidence measurement of annihilation radiation for providing chemical state information; the observations have been corroborated by angular correlation and Doppler broadening measurements and supplemented by the magnetic quenching in the angular correlation and peak-to-valley ratio in the Ge(Li) singles spectrum for the 511 keV line. (author)

  17. Peculiarities of the early Universe (Universes) birth and positron annihilation

    International Nuclear Information System (INIS)

    Svetlov-Prokop'ev, E.P.

    2003-01-01

    Works on the problem of quantum birth of the Universe are reviewed. Possible peculiarities of electron-positron annihilation at the early stages of the Universe (s) birth in connection with black holes are considered. Possible concept of Eternity is discussed. (author)

  18. Annihilation of antiprotons stopped in liquid hydrogen and deuterium

    International Nuclear Information System (INIS)

    Dalkarov, O.D.; Kerbikov, B.O.; Markushin, V.E.

    1976-01-01

    Detailed analysis is given of stopping antiproton annihilation in liquid hydrogen and deuterium. Connection between capture schedule and properties of bound states in nucleon-antinucleon system is established. The theoretical predictions are compared with experimental data which appeared in 1971-75

  19. The electroweak interaction in e+e- annihilations

    International Nuclear Information System (INIS)

    Marshall, R.

    1982-04-01

    The role of e + e - annihilation in studying the weak neutral current, at PETRA and PEP, is reviewed. The way in which the vector and axial vector couplings appear in the total cross sections, the angular distributions and the polarisation dependences are discussed. The dependence of external gauge models on the results of PETRA and PEP experiments is examined. (U.K.)

  20. Hidden strangeness production in two body nbarp annihilation in flight

    CERN Document Server

    Filippi, A

    1999-01-01

    The relative production rates of the final states phi pi sup + , omega pi sup + , eta pi sup + , eta'pi sup + in nbarp annihilation in flight are studied in order to check OZI rule violation effects in both the vectorial and pseudoscalar sectors.

  1. Positron Annihilation in a Rubber Modified Epoxy Resin

    DEFF Research Database (Denmark)

    Mogensen, O. E.; Jacobsen, F. M.; Pethrick, R. A.

    1979-01-01

    Positron annihilation data is reported on a rubber-modified epoxy resin. Studies of the temperature dependence of the o-positronium lifetime indicated the existence of three distinct regions; the associated transition temperatures by comparison with dilatometric data can be ascribed respectively...

  2. Positron annihilation and tribological studies of nano-embedded Al ...

    Indian Academy of Sciences (India)

    Positron annihilation studies of aluminium alloys with nanodispersions of insoluble elements, i.e., In, Sn, Pb and Au were reported. The alloys were obtained using a rapid solidification process. For all alloys, except that with Au, the average diameter of nanoparticles in aluminium matrix was 100 nm, and variance of the size ...

  3. Positron annihilation in vacancies at grain boundaries in metals

    Czech Academy of Sciences Publication Activity Database

    Kuriplach, J.; Melikhova, O.; Hou, M.; Van Petegem, S.; Zhurkin, E.; Šob, Mojmír

    2008-01-01

    Roč. 255, č. 1 (2008), s. 128-132 ISSN 0169-4332 R&D Projects: GA MŠk OC 147; GA AV ČR IAA1041302 Institutional research plan: CEZ:AV0Z20410507 Keywords : Positron annihilation * Grain boundaries * Vacancies Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.576, year: 2008

  4. Is positron annihilation in polyamide 6 affected by morphology?

    Czech Academy of Sciences Publication Activity Database

    Debowska, M.; Piglowski, J.; Slusarczyk, C.; Schmidt, Pavel; Rudzinska-Girulska, J.; Suzuki, T.; Yu, R.; Binias, W.

    2005-01-01

    Roč. 132, SI (2005), s. 64-68 ISSN 1230-3666. [International Conference on X-Ray Investigation of Polymer Structure /6./. Bielsko-Biala, 08.12.2004-11.12.2004] Institutional research plan: CEZ:AV0Z40500505 Keywords : polyamide 6 * crystalline regions * positron annihilation Subject RIV: CD - Macromolecular Chemistry Impact factor: 0.397, year: 2005

  5. World View, the University Establishment, and Cultural Annihilation

    Science.gov (United States)

    Toelken, Barre

    1975-01-01

    Suggests that in the name of liberalism, the social system annihilates other cultures by ensuring that only their sellouts can get on in the world while the subjects and processes which could more fully inform the academic process is ignored. (Author/AM)

  6. Invariant Distributionally Scrambled Manifolds for an Annihilation Operator

    Directory of Open Access Journals (Sweden)

    Xinxing Wu

    2014-01-01

    Full Text Available This note proves that the annihilation operator of a quantum harmonic oscillator admits an invariant distributionally ε-scrambled linear manifold for any 0<ε<2. This is a positive answer to Question 1 by Wu and Chen (2013.

  7. Modelling of Excess Vacancy Annihilation at Different Types of Sinks

    Czech Academy of Sciences Publication Activity Database

    Fischer, F. D.; Svoboda, Jiří; Appel, F.; Kozeschnik, E.

    2011-01-01

    Roč. 59, č. 9 (2011), s. 3463-3472 ISSN 1359-6454 R&D Projects: GA ČR GAP108/10/1781 Institutional research plan: CEZ:AV0Z20410507 Keywords : Vacancies * Annihilation * Substitutional diffusion Subject RIV: BJ - Thermodynamics Impact factor: 3.755, year: 2011

  8. Noncolocated Structural Vibration Suppression Using Zero Annihilation Periodic Control

    Science.gov (United States)

    Bayard, David S.; Boussalis, Dhemetrios

    1993-01-01

    The Zero Annihilation Periodic (ZAP) controller is applied to the problem of vibration control of a noncolocated flexible structure. It is shown that even though the transfer function is nonminimum-phase, a plant inverse controller can be designed which elicits a deadbeat closed-loop response.

  9. Integrodifferential formulations of the continuous-time random walk for solute transport subject to bimolecular A +B →0 reactions: From micro- to mesoscopic

    Science.gov (United States)

    Hansen, Scott K.; Berkowitz, Brian

    2015-03-01

    We develop continuous-time random walk (CTRW) equations governing the transport of two species that annihilate when in proximity to one another. In comparison with catalytic or spontaneous transformation reactions that have been previously considered in concert with CTRW, both species have spatially variant concentrations that require consideration. We develop two distinct formulations. The first treats transport and reaction microscopically, potentially capturing behavior at sharp fronts, but at the cost of being strongly nonlinear. The second, mesoscopic, formulation relies on a separation-of-scales technique we develop to separate microscopic-scale reaction and upscaled transport. This simplifies the governing equations and allows treatment of more general reaction dynamics, but requires stronger smoothness assumptions of the solution. The mesoscopic formulation is easily tractable using an existing solution from the literature (we also provide an alternative derivation), and the generalized master equation (GME) for particles undergoing A +B →0 reactions is presented. We show that this GME simplifies, under appropriate circumstances, to both the GME for the unreactive CTRW and to the advection-dispersion-reaction equation. An additional major contribution of this work is on the numerical side: to corroborate our development, we develop an indirect particle-tracking-partial-integro-differential-equation (PIDE) hybrid verification technique which could be applicable widely in reactive anomalous transport. Numerical simulations support the mesoscopic analysis.

  10. The characterization of the gamma-ray signal from the central Milky Way: A case for annihilating dark matter

    Science.gov (United States)

    Daylan, Tansu; Finkbeiner, Douglas P.; Hooper, Dan; Linden, Tim; Portillo, Stephen K. N.; Rodd, Nicholas L.; Slatyer, Tracy R.

    2016-06-01

    Past studies have identified a spatially extended excess of ˜1-3 GeV gamma rays from the region surrounding the Galactic Center, consistent with the emission expected from annihilating dark matter. We revisit and scrutinize this signal with the intention of further constraining its characteristics and origin. By applying cuts to the Fermi event parameter CTBCORE, we suppress the tails of the point spread function and generate high resolution gamma-ray maps, enabling us to more easily separate the various gamma-ray components. Within these maps, we find the GeV excess to be robust and highly statistically significant, with a spectrum, angular distribution, and overall normalization that is in good agreement with that predicted by simple annihilating dark matter models. For example, the signal is very well fit by a 36-51 GeV dark matter particle annihilating to b b ¯ with an annihilation cross section of σv =(1 - 3) × 10-26cm3 / s (normalized to a local dark matter density of 0.4 GeV /cm3). Furthermore, we confirm that the angular distribution of the excess is approximately spherically symmetric and centered around the dynamical center of the Milky Way (within ˜ 0.05∘ of Sgr A∗), showing no sign of elongation along the Galactic Plane. The signal is observed to extend to at least ≃ 10∘ from the Galactic Center, which together with its other morphological traits disfavors the possibility that this emission originates from previously known or modeled pulsar populations.

  11. Switching and sensing spin states of co-porphyrin in bimolecular reactions on Au111 using scanning tunneling microscopy.

    Science.gov (United States)

    Kim, Howon; Chang, Yun Hee; Lee, Soon-Hyeong; Kim, Yong-Hyun; Kahng, Se-Jong

    2013-10-22

    Controlling and sensing spin states of magnetic molecules at the single-molecule level is essential for spintronic molecular device applications. Here, we demonstrate that spin states of Co-porphyrin on Au(111) can be reversibly switched over by binding and unbinding of the NO molecule and can be sensed using scanning tunneling microscopy and spectroscopy (STM and STS). Before NO exposure, Co-porphryin showed a clear zero-bias peak, a signature of Kondo effect in STS, whereas after NO exposures, it formed a molecular complex, NO-Co-porphyrin, that did not show any zero-bias feature, implying that the Kondo effect was switched off by binding of NO. The Kondo effect could be switched back on by unbinding of NO through single-molecule manipulation or thermal desorption. Our density functional theory calculation results explain the observations with pairing of unpaired spins in dz(2) and ppπ* orbitals of Co-porphyrin and NO, respectively. Our study opens up ways to control molecular spin state and Kondo effect by means of enormous variety of bimolecular binding and unbinding reactions on metallic surfaces.

  12. Gateway Vectors for Simultaneous Detection of Multiple Protein-Protein Interactions in Plant Cells Using Bimolecular Fluorescence Complementation.

    Science.gov (United States)

    Kamigaki, Akane; Nito, Kazumasa; Hikino, Kazumi; Goto-Yamada, Shino; Nishimura, Mikio; Nakagawa, Tsuyoshi; Mano, Shoji

    2016-01-01

    Bimolecular fluorescence complementation (BiFC) is widely used to detect protein-protein interactions, because it is technically simple, convenient, and can be adapted for use with conventional fluorescence microscopy. We previously constructed enhanced yellow fluorescent protein (EYFP)-based Gateway cloning technology-compatible vectors. In the current study, we generated new Gateway cloning technology-compatible vectors to detect BiFC-based multiple protein-protein interactions using N- and C-terminal fragments of enhanced cyan fluorescent protein (ECFP), enhanced green fluorescent protein (EGFP), and monomeric red fluorescent protein (mRFP1). Using a combination of N- and C-terminal fragments from ECFP, EGFP and EYFP, we observed a shift in the emission wavelength, enabling the simultaneous detection of multiple protein-protein interactions. Moreover, we developed these vectors as binary vectors for use in Agrobacterium infiltration and for the generate transgenic plants. We verified that the binary vectors functioned well in tobacco cells. The results demonstrate that the BiFC vectors facilitate the design of various constructions and are convenient for the detection of multiple protein-protein interactions simultaneously in plant cells.

  13. Gateway Vectors for Simultaneous Detection of Multiple Protein−Protein Interactions in Plant Cells Using Bimolecular Fluorescence Complementation

    Science.gov (United States)

    Hikino, Kazumi; Goto-Yamada, Shino; Nishimura, Mikio; Nakagawa, Tsuyoshi; Mano, Shoji

    2016-01-01

    Bimolecular fluorescence complementation (BiFC) is widely used to detect protein—protein interactions, because it is technically simple, convenient, and can be adapted for use with conventional fluorescence microscopy. We previously constructed enhanced yellow fluorescent protein (EYFP)-based Gateway cloning technology-compatible vectors. In the current study, we generated new Gateway cloning technology-compatible vectors to detect BiFC-based multiple protein—protein interactions using N- and C-terminal fragments of enhanced cyan fluorescent protein (ECFP), enhanced green fluorescent protein (EGFP), and monomeric red fluorescent protein (mRFP1). Using a combination of N- and C-terminal fragments from ECFP, EGFP and EYFP, we observed a shift in the emission wavelength, enabling the simultaneous detection of multiple protein—protein interactions. Moreover, we developed these vectors as binary vectors for use in Agrobacterium infiltration and for the generate transgenic plants. We verified that the binary vectors functioned well in tobacco cells. The results demonstrate that the BiFC vectors facilitate the design of various constructions and are convenient for the detection of multiple protein—protein interactions simultaneously in plant cells. PMID:27490375

  14. The influence of the "cage effect" on the mechanism of reversible bimolecular multistage chemical reactions in solutions.

    Science.gov (United States)

    Doktorov, Alexander B

    2015-08-21

    Manifestations of the "cage effect" at the encounters of reactants are theoretically treated by the example of multistage reactions in liquid solutions including bimolecular exchange reactions as elementary stages. It is shown that consistent consideration of quasi-stationary kinetics of multistage reactions (possible only in the framework of the encounter theory) for reactions proceeding near reactants contact can be made on the basis of the concepts of a "cage complex." Though mathematically such a consideration is more complicated, it is more clear from the standpoint of chemical notions. It is established that the presence of the "cage effect" leads to some important effects not inherent in reactions in gases or those in solutions proceeding in the kinetic regime, such as the appearance of new transition channels of reactant transformation that cannot be caused by elementary event of chemical conversion for the given mechanism of reaction. This results in that, for example, rate constant values of multistage reaction defined by standard kinetic equations of formal chemical kinetics from experimentally measured kinetics can differ essentially from real values of these constants.

  15. Bimolecular Complementation to Visualize Filovirus VP40-Host Complexes in Live Mammalian Cells: Toward the Identification of Budding Inhibitors

    Directory of Open Access Journals (Sweden)

    Yuliang Liu

    2011-01-01

    Full Text Available Virus-host interactions play key roles in promoting efficient egress of many RNA viruses, including Ebola virus (EBOV or “e” and Marburg virus (MARV or “m”. Late- (L- domains conserved in viral matrix proteins recruit specific host proteins, such as Tsg101 and Nedd4, to facilitate the budding process. These interactions serve as attractive targets for the development of broad-spectrum budding inhibitors. A major gap still exists in our understanding of the mechanism of filovirus budding due to the difficulty in detecting virus-host complexes and mapping their trafficking patterns in the natural environment of the cell. To address this gap, we used a bimolecular complementation (BiMC approach to detect, localize, and follow the trafficking patterns of eVP40-Tsg101 complexes in live mammalian cells. In addition, we used the BiMC approach along with a VLP budding assay to test small molecule inhibitors identified by in silico screening for their ability to block eVP40 PTAP-mediated interactions with Tsg101 and subsequent budding of eVP40 VLPs. We demonstrated the potential broad spectrum activity of a lead candidate inhibitor by demonstrating its ability to block PTAP-dependent binding of HIV-1 Gag to Tsg101 and subsequent egress of HIV-1 Gag VLPs.

  16. Study of $ \\bar{p} $ and $ \\bar{n} $ annihilations at LEAR with OBELIX, a large acceptance and high resolution detector based on the Open Axial Field Spectrometer

    CERN Multimedia

    2002-01-01

    % PS201 Study of $\\bar{p}$ and $\\bar{n}$ annihilations at LEAR with OBELIX, a large acceptance and high resolution detector based on the Open Axial Field Spectrometer \\\\ \\\\OBELIX is designed to study exclusive final states of antiproton and antineutron annihilations at low energies with protons and nuclei. \\\\ \\\\The physics motivations of the experiment are:\\\\ \\\\\\begin{itemize} \\item (gg, ggg), hybrids ($ q \\bar{q} g $), multiquarks ($ q q \\bar{q} \\bar{q} $) and light mesons ($ q \\bar{q} $) produced in $ N \\bar{N} $ annihilations and study of their spectroscopy and decays. Also broad structures will be searched for by comparing identical decay modes in exclusive final states of the same type occuring from initial states with different angular momentum or isospin. \\item Study of the dynamics of $ N \\bar{N} $ interactions and of the dependence of the final and intermediate resonant states of annihilation upon the quantum numbers of the initial $ N \\bar{N} $ state (angular momentum: S and P-wave in $\\bar{p}p $ at...

  17. Dark matter distribution and annihilation at the Galactic center

    International Nuclear Information System (INIS)

    Dokuchaev, V I; Eroshenko, Yu N

    2016-01-01

    We describe a promising method for measuring the total dark matter mass near a supermassive black hole at the Galactic center based on observations of nonrelativistic precession of the orbits of fast S0 stars. An analytical expression for the precession angle has been obtained under the assumption of a power-law profile of the dark matter density. The awaited weighing of the dark matter at the Galactic center provides the strong constraints on the annihilation signal from the neuralino dark matter particle candidate. The mass of the dark matter necessary for the explanation of the observed excess of gamma-radiation owing to the annihilation of the dark matter particles has been calculated with allowance for the Sommerfeld effect. (paper)

  18. Appearance of a Minimal Length in $e^+ e^-$ Annihilation

    CERN Document Server

    Dymnikova, Irina; Ulbricht, Jürgen

    2014-01-01

    Experimental data reveal with a 5$\\sigma$ significance the existence of a characteristic minimal length $l_e$= 1.57 × 10$^{−17}$ cm at the scale E = 1.253 TeV in the annihilation reaction $e^+e^- \\to \\gamma\\gamma(\\gamma)$ . Nonlinear electrodynamics coupled to gravity and satisfying the weak energy condition predicts, for an arbitrary gauge invariant Lagrangian, the existence of spinning charged electromagnetic soliton asymptotically Kerr-Newman for a distant observer with the gyromagnetic ratio g=2 . Its internal structure includes a rotating equatorial disk of de Sitter vacuum which has properties of a perfect conductor and ideal diamagnetic, displays superconducting behavior, supplies a particle with the finite positive electromagnetic mass related to breaking of space-time symmetry, and gives some idea about the physical origin of a minimal length in annihilation.

  19. Influence of substituents on positron annihilation in styrene copolymers

    International Nuclear Information System (INIS)

    Baranowski, A.; Debowska, M.; Jerie, K.; Rudzinska-Girulska, J.

    1995-01-01

    Results of angular correlation of annihilation radiation (ACAR) and positron annihilation lifetime (PAL) measurements are presented for five styrene copolymers: poly(co-styrene-phenylmaleimide) and its three derivatives with chlorine as well as for one with the OH group substituted at the benzene ring. It occurs that the chlorine substituted at three different positions at the benzene ring poly(co-styrene-o (or -m,-p)-chlorophenylmaleimide) inhibits the formation of the positronium to different extent. The greatest effect is observed in case of the chlorine atom substituted at the benzene ring at the ortho-position towards the nitrogen atom. The two long lifetime (τ 3 and τ 4 ) observed in the lifetime spectra are connected with the bimodal distributions of the free volume radius in the samples. (author) 13 refs.; 3 figs.; 3 tabs

  20. Positron annihilation studies of some charge transfer molecular complexes

    CERN Document Server

    El-Sayed, A; Boraei, A A A

    2000-01-01

    Positron annihilation lifetimes were measured for some solid charge transfer (CT) molecular complexes of quinoline compounds (2,6-dimethylquinoline, 6-methoxyquinoline, quinoline, 6-methylquinoline, 3-bromoquinoline and 2-chloro-4-methylquinoline) as electron donor and picric acid as an electron acceptor. The infrared spectra (IR) of the solid complexes clearly indicated the formation of the hydrogen-bonding CT-complexes. The annihilation spectra were analyzed into two lifetime components using PATFIT program. The values of the average and bulk lifetimes divide the complexes into two groups according to the non-bonding ionization potential of the donor (electron donating power) and the molecular weight of the complexes. Also, it is found that the ionization potential of the donors and molecular weight of the complexes have a conspicuous effect on the average and bulk lifetime values. The bulk lifetime values of the complexes are consistent with the formation of stable hydrogen-bonding CT-complexes as inferred...

  1. Gamma rays from the annihilation of singlet scalar dark matter

    Science.gov (United States)

    Yaguna, Carlos E.

    2009-03-01

    We consider an extension of the Standard Model by a singlet scalar that accounts for the dark matter of the Universe. Within this model we compute the expected gamma ray flux from the annihilation of dark matter particles in a consistent way. To do so, an updated analysis of the parameter space of the model is first presented. By enforcing the relic density constraint from the very beginning, the viable parameter space gets reduced to just two variables: the singlet mass and the higgs mass. Current direct detection constraints are then found to require a singlet mass larger than 50 GeV. Finally, we compute the gamma ray flux and annihilation cross section and show that a large fraction of the viable parameter space lies within the sensitivity of Fermi-GLAST.

  2. High nuclear temperatures by antimatter-matter annihilation

    International Nuclear Information System (INIS)

    Gibbs, W.R.; Strottman, D.

    1985-01-01

    It is suggested that the quark-gluon phase be created through the use of antiproton or antideuteron beams. The first advantage to this method, using higher energy antiprotons than 1.5 GeV/c, is that the higher momenta antiprotons penetrate more deeply so that mesons produced are more nearly contained within the nucleus. Another advantage is that the annihilation products are very forward-peaked and tend to form a beam of mesons so that the energy density does not disperse very rapidly. Calculations were performed using the intranuclear cascade to try to follow the process of annihilation in some detail. The intranuclear cascade type calculation method is compared to the hydrodynamic approach. 8 refs., 8 figs

  3. Gamma rays from the annihilation of singlet scalar dark matter

    International Nuclear Information System (INIS)

    Yaguna, Carlos E.

    2009-01-01

    We consider an extension of the Standard Model by a singlet scalar that accounts for the dark matter of the Universe. Within this model we compute the expected gamma ray flux from the annihilation of dark matter particles in a consistent way. To do so, an updated analysis of the parameter space of the model is first presented. By enforcing the relic density constraint from the very beginning, the viable parameter space gets reduced to just two variables: the singlet mass and the higgs mass. Current direct detection constraints are then found to require a singlet mass larger than 50 GeV. Finally, we compute the gamma ray flux and annihilation cross section and show that a large fraction of the viable parameter space lies within the sensitivity of Fermi-GLAST

  4. Beyond 'invisibility': queer intelligibility and symbolic annihilation in healthcare.

    Science.gov (United States)

    Müller, Alex

    2018-01-01

    Sexual minority health is increasingly receiving attention by health sciences education and healthcare, with the core argument being that health can be improved by challenging sexual minority invisibility. Invisibility as a concept, however, does not allow for a deeper theoretical engagement with the reasons and consequences of the lack of representation of queerness in healthcare. Drawing on empirical research with queer healthcare users in South Africa, I argue that 'invisibility' actually encompasses two distinct, though related, concepts: queer symbolic annihilation as the reason for the exclusion of queer identities in health professions education and, by consequence, in healthcare; and queer (un)intelligibility as the consequence of this systemic erasure. By simply attributing discriminatory healthcare experiences of queer people to 'invisibility' we are missing opportunities to address underlying issues of queer symbolic annihilation and unintelligibility.

  5. Exciton–exciton annihilation and biexciton stimulated emission in graphene nanoribbons

    Science.gov (United States)

    Soavi, Giancarlo; Dal Conte, Stefano; Manzoni, Cristian; Viola, Daniele; Narita, Akimitsu; Hu, Yunbin; Feng, Xinliang; Hohenester, Ulrich; Molinari, Elisa; Prezzi, Deborah; Müllen, Klaus; Cerullo, Giulio

    2016-01-01

    Graphene nanoribbons display extraordinary optical properties due to one-dimensional quantum-confinement, such as width-dependent bandgap and strong electron–hole interactions, responsible for the formation of excitons with extremely high binding energies. Here we use femtosecond transient absorption spectroscopy to explore the ultrafast optical properties of ultranarrow, structurally well-defined graphene nanoribbons as a function of the excitation fluence, and the impact of enhanced Coulomb interaction on their excited states dynamics. We show that in the high-excitation regime biexcitons are formed by nonlinear exciton–exciton annihilation, and that they radiatively recombine via stimulated emission. We obtain a biexciton binding energy of ≈250 meV, in very good agreement with theoretical results from quantum Monte Carlo simulations. These observations pave the way for the application of graphene nanoribbons in photonics and optoelectronics. PMID:26984281

  6. Comments on charm production in electron positron annihilation

    International Nuclear Information System (INIS)

    Close, F.E.

    1976-09-01

    The circumstances are discussed in which the production of D anti D: DD*: D* anti D* in electron positron annihilation is expected to be in the ratio 1:4:7 suggested by counting the available spin states. The physical significance of the requisite assumptions is discussed. The importance of taking into account the finite detector acceptance is stressed and tests for a possible 3 D 1 component in the D* are proposed. (author)

  7. Positron Annihilation Spectroscopy study of minerals commonly found in shale

    Science.gov (United States)

    Alsleben, Helge; Ameena, Fnu; Bufkin, James; Chun, Joah; Quarles, C. A.

    2018-01-01

    Positron Annihilation Lifetime and Doppler Broadening spectroscopies are used to investigate twenty-three different rock-forming minerals that are commonly found in shale. Doppler Broadening provides information about the positron and positronium (Ps) trapping sites for comparison among the various minerals. Correlations of positron lifetime and Doppler Broadening are observed for different groups of minerals. Finally, Ps formation, or lack thereof, in the various minerals has been determined.

  8. Multiwavelength analysis of dark matter annihilation and RX-DMFIT

    Energy Technology Data Exchange (ETDEWEB)

    McDaniel, A.; Jeltema, T.; Profumo, S. [Department of Physics, University of California, 1156 High St. Santa Cruz, CA, 95064 (United States); Storm, E., E-mail: alexmcdaniel@ucsc.edu, E-mail: tesla@ucsc.edu, E-mail: profumo@ucsc.edu, E-mail: e.m.storm@uva.nl [GRAPPA, Institute of Physics, Universiteit van Amsterdam Science Park 904, 1098XH Amsterdam (Netherlands)

    2017-09-01

    Dark matter (DM) particles are predicted by several well motivated models to yield Standard Model particles through self-annihilation that can potentially be detected by astrophysical observations. In particular, the production of charged particles from DM annihilation in astrophysical systems that contain magnetic fields yields radio emission through synchrotron radiation and X-ray emission through inverse Compton scattering of ambient photons. We introduce RX-DMFIT, a tool used for calculating the expected secondary emission from DM annihilation. RX-DMFIT includes a wide range of customizable astrophysical and particle parameters and incorporates important astrophysics including the diffusion of charged particles, relevant radiative energy losses, and magnetic field modelling. We demonstrate the use and versatility of RX-DMFIT by analyzing the potential radio and X-ray signals for a variety of DM particle models and astrophysical environments including galaxy clusters, dwarf spheroidal galaxies and normal galaxies. We then apply RX-DMFIT to a concrete example using Segue I radio data to place constraints for a range of assumed DM annihilation channels. For WIMP models with M {sub χ} ≤ 100 GeV and assuming weak diffusion, we find that the leptonic μ{sup +}μ{sup −} and τ{sup +}τ{sup −} final states provide the strongest constraints, placing limits on the DM particle cross-section well below the thermal relic cross-section, while even for the b b-bar channel we find limits close to the thermal relic cross-section. Our analysis shows that radio emission provides a highly competitive avenue for dark matter searches.

  9. Annihilators in infinite-dimensional Grassmann-Banach algebras

    International Nuclear Information System (INIS)

    Ivashchuk, V.D.

    1989-01-01

    A family of infinite-dimensional Grassmann-Banach algebras over a complete normed field K is considered. It is shown that every element G of the family is an associative supercommutative Banach superalgebra over K: G double-bond G 0 circle-plus G 1 with zero annihilators G 0 perpendicular double-bond G 1 perpendicular double-bond(G 1 (κ) ) perpendicular double-bond(0), k ≥ 2

  10. Experimental study of jets in electron-positron-annihilation

    International Nuclear Information System (INIS)

    Bartel, W.; Cords, D.; Dittmann, P.; Eichler, R.; Felst, R.; Haidt, D.; Krehbiel, H.; Naroska, B.; O'Neill, L.H.; Steffen, P.

    1981-02-01

    Data on hadron production by e + e - -annihilation at c.m. energies between 30 GeV and 36 GeV are presented and compared with two models both based on first order QCD but using different schemes for the fragmentation of quarks and gluons into hadrons. In one model the fragmentation proceeds along the parton momenta, in the other along the colour-anticolour axes. The data are reproduced better by fragmentation along the colour axes. (orig.)

  11. Inclusive anomalous muon production in e+e- annihilation

    International Nuclear Information System (INIS)

    Feldman, G.J.; Bulos, F.; Lueke, D.; Abrams, G.S.; Alam, M.S.; Boyarski, A.M.; Breidenbach, M.; Dorfan, J.; Friedberg, C.E.; Fryberger, D.; Goldhaber, G.; Hanson, G.; Heile, F.B.; Jaros, J.A.; Kadyk, J.A.; Larsen, R.R.; Litke, A.M.; Lueth, V.; Madaras, R.J.; Morehouse, C.C.; Nguyen, H.K.; Paterson, J.M.; Perl, M.L.; Peruzzi, I.; Piccolo, M.; Pierre, F.M.; Pun, T.P.; Rapidis, P.; Richter, B.; Sadoulet, B.; Schwitters, R.F.; Tanenbaum, W.; Trilling, G.H.; Vannucci, F.; Whitaker, J.S.; Wiss, J.E.

    1977-01-01

    We present measurements of inclusive anomalous muon production in e + e - annihilations in three energy ranges. In all three ranges we observe a large anomalous muon production rate in two-prong events which is compatible with the expected decays of pairs of heavy leptons. In the highest energy range there is also appreciable anomalous muon production in multiprong events which, due to its magnitude and momentum dependence, must come in part from a source other than a heavy lepton

  12. Zero-Annihilation Periodic Control For Damping Vibrations

    Science.gov (United States)

    Bayard, David S.; Boussalis, Dhemetrios

    1995-01-01

    Report presents study on use of recently developed zero-annihilation periodic (ZAP) controller for active suppression of vibrations in flexible structures characterized by non-minimum-phase transfer functions. Non-minimum-phase situation occurs if certain kinds of vibration-sensor/vibration-actuator pairs (e.g., piezoelectric) used, and/or if vibration sensor(s) not colocated with vibration actuator(s).

  13. Investigation of corrosion defects in titanium by positron annihilation

    Directory of Open Access Journals (Sweden)

    Pietrzak Ryszard

    2015-12-01

    Full Text Available The positron annihilation method was used to study the formation of defects in titanium samples during their corrosion in the vapor of a 3% HCl solution. In particular, the distribution of defects depending on the distance from the corroding surface and the impact of an external magnetic field on the concentration of vacancies forming during the corrosion of titanium layers close to the surface were determined.

  14. Production of Higgs bosons and hyperions in e+e- annihilation

    International Nuclear Information System (INIS)

    Ali, A.

    1980-10-01

    The production of hyperions - low lying pseudo-Goldstone modes of the hypercolor scenario - in e + e - annihilation is studied and contrasted with the production of elementary Higgs of the canonical methodology. 1. The possibility of implementing the Higgs mechanism in a dynamical way, without the use of elementary spin-0 fields, has lately been the subject of much discussion. In several recent communications it has been pointed out that the most popular dynamical scheme, the so-called hypercolor scenario, may be experimentally distinguishable from the canonical Weinberg-Salam scheme via experiments at relatively low (10-100 GeV) energies. [There is, of course, an a priori expectation that differences between the two schemes will be manifest in experiments at TeV energies; this energy regime, however is not likely to be accessible in the near future.] The considerations of refs.(2-4) hinge in a crucial way on one's ability to (a) produce spin-O particles, of mass approx. 10 GeV, coupled semi-weakly to ordinary quarks and leptons and (b) distinguish Higgs particles, phi's, from the low-lying bosons of the hypercolor scenario, generically called π's, exploiting mainly the difference in parity. Our purpose in this note is to point out that the pseudosclar nature of π''s introduces a fundamental difference in the production mechanism of phi's and π''s in a large class of reactions. In particular, we calculate the production rates of phi's and π''s in e + e - annihilation and in the decays of the spin-1 bosons Z and toponium, Jsub(T). (orig.)

  15. High sensitivity of positron annihilation to thermal oxidation of polyethylene

    Science.gov (United States)

    Ito, Kenji; Kobayashi, Yoshinori; Nanasawa, Atsushi

    2003-01-01

    We demonstrate the high sensitivity of positron annihilation to compositional changes related to the thermal degradation of polyethylene (PE). Positron annihilation γ-ray and lifetime measurements were conducted for PE films with and without antioxidant (1000-ppm Ciba® IRGANOX® 1076), subjected to heat treatment at 100 °C for different periods, to a maximum of 30 days. For the film without antioxidant, the positron Doppler parameter (S) and ortho-positronium formation probability (Io-Ps) appreciably decreased with increased heat treatment times, whereas they barely changed for the film with antioxidant. This, together with the Fourier transform infrared measurements, demonstrated that the variations of S and Io-Ps are caused by the thermal oxidation of PE. The S parameter was found to be sensitive to the early stage of degradation, where the carbonyl concentration is inferred to be lower than 100 ppm. The high sensitivity results from the large positron mobility in PE and from the high positron affinity of oxygen-containing polar groups. This work provides the basis for an application of positron annihilation to sensitive detection of the initial degradation of PE and other nonpolar polymers.

  16. Search for Dark Matter Annihilation in Galaxy Groups

    Science.gov (United States)

    Lisanti, Mariangela; Mishra-Sharma, Siddharth; Rodd, Nicholas L.; Safdi, Benjamin R.

    2018-03-01

    We use 413 weeks of publicly available Fermi Pass 8 gamma-ray data combined with recently developed galaxy group catalogs to search for evidence of dark matter annihilation in extragalactic halos. In our study, we use luminosity-based mass estimates and mass-to-concentration relations to infer the J factors and associated uncertainties for hundreds of galaxy groups within a redshift range z ≲0.03 . We employ a conservative substructure boost factor model, which only enhances the sensitivity by an O (1 ) factor. No significant evidence for dark matter annihilation is found, and we exclude thermal relic cross sections for dark matter masses below ˜30 GeV to 95% confidence in the b b ¯ annihilation channel. These bounds are comparable to those from Milky Way dwarf spheroidal satellite galaxies. The results of our analysis increase the tension but do not rule out the dark matter interpretation of the Galactic Center excess. We provide a catalog of the galaxy groups used in this study and their inferred properties, which can be broadly applied to searches for extragalactic dark matter.

  17. φ meson production in pp annihilation at rest

    International Nuclear Information System (INIS)

    Srisuphaphon, S.; Yan, Y.; Gutsche, Thomas; Lyubovitskij, Valery E.

    2011-01-01

    Apparent channel-dependent violations of the Okubo-Zwieg-Iizuka (OZI) rule in nucleon-antinucleon annihilation reactions in the presence of an intrinsic strangeness component in the nucleon are discussed. Admixture of ss quark pairs in the nucleon wave function enables the direct coupling to the φ-meson in the annihilation channel without violating the OZI rule. Three forms are considered in this work for the strangeness content of the proton wave function, namely, the uud cluster with a ss sea-quark component, kaon-hyperon clusters based on a simple chiral quark model, and the pentaquark picture uudss. Nonrelativistic quark model calculations reveal that the strangeness magnetic moment μ s and the strangeness contribution to the proton spin σ s from the first two models are consistent with recent experimental data, where μ s and σ s are negative. For the third model, the uuds subsystem with the configurations [31] FS [211] F [22] S and [31] FS [31] F [22] S leads to negative values of μ s and σ s . With effective quark line diagrams incorporating the 3 P 0 model, we give estimates for the branching ratios of the annihilation reactions at rest pp→φX (X=π 0 , η, ρ 0 , ω). Results for the branching ratios of φX production from atomic pp s-wave states are for the first and third model found to be strongly channel dependent, in good agreement with measured rates.

  18. Search for Dark Matter Annihilation in Galaxy Groups.

    Science.gov (United States)

    Lisanti, Mariangela; Mishra-Sharma, Siddharth; Rodd, Nicholas L; Safdi, Benjamin R

    2018-03-09

    We use 413 weeks of publicly available Fermi Pass 8 gamma-ray data combined with recently developed galaxy group catalogs to search for evidence of dark matter annihilation in extragalactic halos. In our study, we use luminosity-based mass estimates and mass-to-concentration relations to infer the J factors and associated uncertainties for hundreds of galaxy groups within a redshift range z≲0.03. We employ a conservative substructure boost factor model, which only enhances the sensitivity by an O(1) factor. No significant evidence for dark matter annihilation is found, and we exclude thermal relic cross sections for dark matter masses below ∼30  GeV to 95% confidence in the bb[over ¯] annihilation channel. These bounds are comparable to those from Milky Way dwarf spheroidal satellite galaxies. The results of our analysis increase the tension but do not rule out the dark matter interpretation of the Galactic Center excess. We provide a catalog of the galaxy groups used in this study and their inferred properties, which can be broadly applied to searches for extragalactic dark matter.

  19. The PAMELA positron excess from annihilations into a light boson

    Energy Technology Data Exchange (ETDEWEB)

    Cholis, Ilias; Goodenough, Lisa; Weiner, Neal [Center for Cosmology and Particle Physics, Department of Physics, New York University, New York, NY 10003 (United States); Finkbeiner, Douglas P., E-mail: ijc219@nyu.edu, E-mail: dfinkbeiner@cfa.harvard.edu, E-mail: lcg261@nyu.edu, E-mail: neal.weiner@nyu.edu [Harvard-Smithsonian Center for Astrophysics, 60 Garden St., Cambridge, MA 02138 (United States)

    2009-12-01

    Recently published results from the PAMELA experiment have shown conclusive evidence for an excess of positrons at high ( ∼ 10–100 GeV) energies, confirming earlier indications from HEAT and AMS-01. Such a signal is generally expected from dark matter annihilations. However, the hard positron spectrum and large amplitude are difficult to achieve in most conventional WIMP models. The absence of any associated excess in anti-protons is highly constraining on models with hadronic annihilation modes. We revisit an earlier proposal, wherein the dark matter annihilates into a new light (∼

  20. Compton-backscattered annihilation radiation from the Galactic Center region

    Science.gov (United States)

    Smith, D. M.; Lin, R. P.; Feffer, P.; Slassi, S.; Hurley, K.; Matteson, J.; Bowman, H. B.; Pelling, R. M.; Briggs, M.; Gruber, D.

    1993-01-01

    On 1989 May 22, the High Energy X-ray and Gamma-ray Observatory for Nuclear Emissions, a balloon-borne high-resolution germanium spectrometer with an 18-deg FOV, observed the Galactic Center (GC) from 25 to 2500 keV. The GC photon spectrum is obtained from the count spectrum by a model-independent method which accounts for the effects of passive material in the instrument and scattering in the atmosphere. Besides a positron annihilation line with a flux of (10.0 +/- 2.4) x 10 exp -4 photons/sq cm s and a full width at half-maximum (FWHM) of (2.9 + 1.0, -1.1) keV, the spectrum shows a peak centered at (163.7 +/- 3.4) keV with a flux of (1.55 +/- 0.47) x 10 exp -3 photons/sq cm s and a FWHM of (24.4 +/- 9.2) keV. The energy range 450-507 keV shows no positronium continuum associated with the annihilation line, with a 2-sigma upper limit of 0.90 on the positronium fraction. The 164 keV feature is interpreted as Compton backscatter of broadened and redshifted annihilation radiation, possibly from the source 1E 1740.7-2942.

  1. Effect of micellar environment on Marcus correlation curves for photoinduced bimolecular electron transfer reactions

    Science.gov (United States)

    Kumbhakar, Manoj; Nath, Sukhendu; Mukherjee, Tulsi; Pal, Haridas

    2005-07-01

    Photoinduced electron transfer (ET) between coumarin dyes and aromatic amine has been investigated in two cationic micelles, namely, cetyltrimethyl ammonium bromide (CTAB) and dodecyltrimethyl ammonium bromide (DTAB), and the results have been compared with those observed earlier in sodium dodecyl sulphate (SDS) and triton-X-100 (TX-100) micelles for similar donor-acceptor pairs. Due to a reasonably high effective concentration of the amines in the micellar Stern layer, the steady-state fluorescence results show significant static quenching. In the time-resolved (TR) measurements with subnanosecond time resolution, contribution from static quenching is avoided. Correlations of the dynamic quenching constants (kqTR), as estimated from the TR measurements, show the typical bell-shaped curves with the free-energy changes (ΔG0) of the ET reactions, as predicted by the Marcus outersphere ET theory. Comparing present results with those obtained earlier for similar coumarin-amine systems in SDS and TX-100 micelles, it is seen that the inversion in the present micelles occurs at an exergonicity (-ΔG0>˜1.2-1.3eV) much higher than that observed in SDS and TX-100 micelles (-ΔG0>˜0.7eV), which has been rationalized based on the relative propensities of the ET and solvation rates in different micelles. In CTAB and DTAB micelles, the kqTR values are lower than the solvation rates, which result in the full contribution of the solvent reorganization energy (λs) towards the activation barrier for the ET reaction. Contrary to this, in SDS and TX-100 micelles, kqTR values are either higher or comparable with the solvation rates, causing only a partial contribution of λs in these cases. Thus, Marcus inversion in present cationic micelles is inferred to be the true inversion, whereas that in the anionic SDS and neutral TX-100 micelles are understood to be the apparent inversion, as envisaged from two-dimensional ET theory.

  2. In vitro visualization and characterization of wild type and mutant IDH homo- and heterodimers using Bimolecular Fluorescence Complementation.

    Science.gov (United States)

    Robinson, Gemma L; Philip, Beatrice; Guthrie, Matthew R; Cox, James E; Robinson, James P; VanBrocklin, Matthew W; Holmen, Sheri L

    2016-05-01

    Mutations in the metabolic enzyme isocitrate dehydrogenase (IDH) were recently found in ~80% of WHO grade II-III gliomas and secondary glioblastomas. These mutations reduce the enzyme's ability to convert isocitrate to α-ketoglutarate and, instead, confer a novel gain-of-function resulting in the conversion of α-ketoglutarate to 2-hydroxglutarate (2-HG). However, IDH mutations exist in a heterozygous state such that a functional wild type allele is retained. Recent data suggest that the ability of mutant IDH1, but not mutant IDH2, to produce 2-HG is dependent on the activity of the retained wild type allele. In this study, we aimed to further our understanding of the interaction and function of wild type and mutant IDH heterodimers utilizing Bimolecular Fluorescence Complementation (BiFC). Dimerization of wild type and mutant IDH monomers conjugated to the N- and C-terminus of Venus protein, respectively, is directly proportional to the amount of fluorescence emitted and can be used as an approach to visualize and assess IDH dimerization. Thus, we utilized this method to visualize IDH homo- and heterodimers and to examine their cellular physiology based on subcellular localization, NADPH production, and 2-HG levels. Our results demonstrate that wild type and mutant IDH1 or IDH2 heterodimers display similar physiological characteristics to that of mutant IDH1 or IDH2 homodimers with the exception of their ability to generate NADPH. IDH1 heterodimers consistently generate NADPH whereas IDH2 heterodimers do not. However, the presence of mutant IDH1 or IDH2 in homo- or heterodimer configurations consistently generates equivalent levels of 2-HG. Our data suggest that the wild type protein is not required for the generation of 2-HG.

  3. One-photon annihilation of thermal positrons with bound atomic electrons

    Science.gov (United States)

    Jung, Young-Dae

    1994-01-01

    Direct one-photon annihilation rate of positrons with a bound atomic electron is evaluated in the nonrelativistic limit. The K- and L-shell contributions are estimated including the screening and effective Coulomb repulsion effects. The annihilation rate of thermal positrons is calculated for various temperatures. The total number of one-photon annihilation events in the interstellar medium is discussed. These results provide the directional and structural information for cosmic gamma-ray sources.

  4. Simulation of the annihilation emission of galactic positrons; Modelisation de l'emission d'annihilation des positrons Galactiques

    Energy Technology Data Exchange (ETDEWEB)

    Gillard, W

    2008-01-15

    Positrons annihilate in the central region of our Galaxy. This has been known since the detection of a strong emission line centered on an energy of 511 keV in the direction of the Galactic center. This gamma-ray line is emitted during the annihilation of positrons with electrons from the interstellar medium. The spectrometer SPI, onboard the INTEGRAL observatory, performed spatial and spectral analyses of the positron annihilation emission. This thesis presents a study of the Galactic positron annihilation emission based on models of the different interactions undergone by positrons in the interstellar medium. The models are relied on our present knowledge of the properties of the interstellar medium in the Galactic bulge, where most of the positrons annihilate, and of the physics of positrons (production, propagation and annihilation processes). In order to obtain constraints on the positrons sources and physical characteristics of the annihilation medium, we compared the results of the models to measurements provided by the SPI spectrometer. (author)

  5. High energy resolution and first time-dependent positron annihilation induced Auger electron spectroscopty

    International Nuclear Information System (INIS)

    Mayer, Jakob

    2010-01-01

    It was the aim of this thesis to improve the existing positron annihilation induced Auger spectrometer at the highly intense positron source NEPOMUC (NEutron induced POsitron source MUniCh) in several ways: Firstly, the measurement time for a single spectrum should be reduced from typically 12 h to roughly 1 h or even less. Secondly, the energy resolution, which amounted to ΔE/E∼10%, should be increased by at least one order of magnitude in order to make high resolution positron annihilation induced Auger spectroscopy (PAES)-measurements of Auger transitions possible and thus deliver more information about the nature of the Auger process. In order to achieve these objectives, the PAES spectrometer was equipped with a new electron energy analyzer. For its ideal operation all other components of the Auger analysis chamber had to be adapted. Particularly the sample manipulation and the positron beam guidance had to be renewed. Simulations with SIMION registered ensured the optimal positron lens parameters. After the adjustment of the new analyzer and its components, first measurements illustrated the improved performance of the PAES setup: Firstly, the measurement time for short overview measurements was reduced from 3 h to 420 s. The measurement time for more detailed Auger spectra was shortened from 12 h to 80 min. Secondly, even with the reduced measurement time, the signal to noise ratio was also enhanced by one order of magnitude. Finally, the energy resolution was improved to ΔE/E 2,3 VV-transition with PAES. Thus, within this thesis two objectives were achieved: Firstly, the PAES spectrometer was renewed and improved by at least one order of magnitude with respect to the signal to noise ratio, the measurement time and the energy resolution. Secondly, several measurements have been carried out, demonstrating the high performance of the spectrometer. Amongst them are first dynamic PAES measurements and a high resolution measurement of the CuM 2,3 VV

  6. Baryon-antibaryon annihilation and reproduction in relativistic heavy-ion collisions

    Science.gov (United States)

    Seifert, E.; Cassing, W.

    2018-02-01

    The quark rearrangement model for baryon-antibaryon annihilation and reproduction (B B ¯↔3 M )—incorporated in the Parton-Hadron-String Dynamics (PHSD) transport approach—is extended to the strangeness sector. A derivation of the transition probabilities for the three-body processes is presented and a strangeness suppression factor for the invariant matrix element squared is introduced to account for the higher mass of the strange quark compared to the light up and down quarks. In simulations of the baryon-antibaryon annihilation and reformation in a box with periodic boundary conditions, we demonstrate that our numerical implementation fulfills detailed balance on a channel-by-channel basis for more than 2000 individual 2 ↔3 channels. Furthermore, we study central Pb+Pb collisions within PHSD from 11.7 A GeV to 158 A GeV and investigate the impact of the additionally implemented reaction channels in the strangeness sector. We find that the new reaction channels have a visible impact essentially only on the rapidity spectra of antibaryons. The spectra with the additional channels in the strangeness sector are closer to the experimental data than without for all antihyperons. Due to the chemical redistribution between baryons-antibaryons and mesons we find a slightly larger production of antiprotons thus moderately overestimating the available experimental data. We additionally address the question if the antibaryon spectra (with strangeness) from central heavy-ion reactions at these energies provide further information on the issue of chiral symmetry restoration and deconfinement. However, by comparing transport results with and without partonic phase as well as including and excluding effects from chiral symmetry restoration we find no convincing signals in the strange antibaryon sector for either transition due to the strong final-state interactions.

  7. Vectors for multi-color bimolecular fluorescence complementation to investigate protein-protein interactions in living plant cells

    Directory of Open Access Journals (Sweden)

    Kuang Lin-Yun

    2008-10-01

    Full Text Available Abstract Background The investigation of protein-protein interactions is important for characterizing protein function. Bimolecular fluorescence complementation (BiFC has recently gained interest as a relatively easy and inexpensive method to visualize protein-protein interactions in living cells. BiFC uses "split YFP" tags on proteins to detect interactions: If the tagged proteins interact, they may bring the two split fluorophore components together such that they can fold and reconstitute fluorescence. The sites of interaction can be monitored using epifluorescence or confocal microscopy. However, "conventional" BiFC can investigate interactions only between two proteins at a time. There are instances when one may wish to offer a particular "bait" protein to several "prey" proteins simultaneously. Preferential interaction of the bait protein with one of the prey proteins, or different sites of interaction between the bait protein and multiple prey proteins, may thus be observed. Results We have constructed a series of gene expression vectors, based upon the pSAT series of vectors, to facilitate the practice of multi-color BiFC. The bait protein is tagged with the C-terminal portion of CFP (cCFP, and prey proteins are tagged with the N-terminal portions of either Venus (nVenus or Cerulean (nCerulean. Interaction of cCFP-tagged proteins with nVenus-tagged proteins generates yellow fluorescence, whereas interaction of cCFP-tagged proteins with nCerulean-tagged proteins generates blue fluorescence. Additional expression of mCherry indicates transfected cells and sub-cellular structures. Using this system, we have determined in both tobacco BY-2 protoplasts and in onion epidermal cells that Agrobacterium VirE2 protein interacts with the Arabidopsis nuclear transport adapter protein importin α-1 in the cytoplasm, whereas interaction of VirE2 with a different importin α isoform, importin α-4, occurs predominantly in the nucleus. Conclusion Multi

  8. Geant4 simulation of annihilation and excitation of positronium

    CERN Document Server

    AUTHOR|(CDS)2156323

    2016-01-01

    The purpose of this report is to document the work done during the summer of 2016 (18/6- 26/8) as a part of the CERN Summer Student Programme. The work has been done at the AEgIS (Antihydrogen Experiment: Gravity, Interferometry, Spectroscopy) collaboration under the supervision of Lillian Smestad and Michael Doser. The goal of the project was to create a Monte Carlo simulation in Geant4, of Positronium annihilation and excitation in the positron test chamber of the AEgIs experiment.

  9. Proton-antiproton annihilation into massive leptons and polarization phenomena

    Energy Technology Data Exchange (ETDEWEB)

    Dbeyssi, A. [Univ. Paris-Sud, CNRS/IN2P3, Institut de Physique Nucleaire, UMR 8608, 91405 Orsay (France); Tomasi-Gustafsson, E., E-mail: etomasi@cea.fr [Univ. Paris-Sud, CNRS/IN2P3, Institut de Physique Nucleaire, UMR 8608, 91405 Orsay (France); Gakh, G.I.; Konchatnyi, M. [National Science Centre, Kharkov Institute of Physics and Technology, 61108 Akademicheskaya 1, Kharkov (Ukraine)

    2012-11-15

    We extend previous calculations of polarization observables for the annihilation reaction p{sup Macron }+p{yields} Script-Small-L {sup -}+ Script-Small-L {sup +} to the case of heavy leptons, such as the {mu}- and {tau}-leptons. We consider the case when the beam and/or the target are polarized, as well as when the outgoing leptons are polarized. We give the dependence of the unpolarized cross section, angular asymmetry, and various polarization observables on the relevant kinematical variables in the center of mass and in the laboratory system, paying particular attention to the effect of the mass induced terms.

  10. Formation of charmonium states in antiproton-proton annihilation

    International Nuclear Information System (INIS)

    Cester, R.

    1984-01-01

    Experiment R704 at the CERN ISR studies charmonium states formed directly in antiproton-proton annihilations. A high luminosity and good centre of mass energy definition are obtained by intersecting a low-energy antiproton beam circulating in ring II at the ISR, with a molecular H 2 jet target. During two test runs, for an integrated luminosity of 265 nb -1 , we have observed formation of psi and chi 2 . Taking the known psi mass as reference, we have checked that the nominal ISR momentum is correct and reproducible to 2.0 MeV/c

  11. Search for heavy neutrinos produced in e+e- annihilation

    International Nuclear Information System (INIS)

    Feldman, G.J.

    1985-05-01

    We report a search for long-lived heavy neutrinos produced by the neutral weak current in e + e - annihilation at 29 GeV at PEP. Data from the Mark II detector are examined for evidence of events with one or more separated vertices in the radial range of 2 mm to 10 cm. No events were found that were consistent with the hypothesis of heavy neutrino production, eliminating the possibility of heavy neutrinos with decay lengths of 1 to 20 cm in mass range 1 to 13 GeV/c 2 . 11 refs

  12. Positron annihilation in the aging alloy Ti49Ni51

    International Nuclear Information System (INIS)

    Baturin, A.A.; Grishkov, V.N.; Lotkov, A.I.

    2002-01-01

    The processes of low temperature aging in alloy Ti 49 Ni 51 at temperatures of 443 and 523 K are investigated using the method of angular correlation of annihilation irradiation. The distinction of positron behaviour in aging TiNi base alloys from that in aging solid solutions on the basis of unalloyed metals is the positron location in type (0001) plane of Ti 3 Ni 4 phase structure which consist practically of nickel atoms only. As this taken place, the parameters of angular correlation spectra are defined by chemical composition of these layers depending on Ti and Ni atoms redistribution between neighboring layers [ru

  13. Positron annihilation study on defects in ion-implanted Si

    International Nuclear Information System (INIS)

    Akahane, T.; Fujinami, M.; Sawada, T.

    2003-01-01

    Two-detector coincidence measurements of the Doppler broadened annihilation spectra with a variable energy positron beam are carried out for the study of the annealing behavior of Si implanted with As, P, Cu and H ions. In P-implanted Si, growth of the defect complexes are observed in coincidence Doppler broadening spectra up to 400degC. In Cu-implanted Si, the formation of defect-Cu complexes is indicated. In H-implanted Si, the passivation effect of hydrogen on positron traps are observed in the low temperature region up to 400degC. (author)

  14. Radiative production of scalar neutrinos in e+e- annihilation

    International Nuclear Information System (INIS)

    Aliev, T.M.; Mustafaev, Kh.A.; Khalil-Zade, F.T.

    1987-01-01

    Radiative production of scalar neutrino pairs in e + e - annihilation is studied in detail in the framework of the R-invariant N=1 supergravity. The doubly differential (with respect to energy and photon emission angle) cross section is calculated. The energy-angular distribution, the photon energy spectra and the total cross section were studied in detail to fit the available experimental conditions. Possibilities of experimental identification of the process under consideration are presented. Restraints vino mass are imposed comparing comparing the obtained results with the data

  15. Positron annihilation lifetime spectroscopy study of roller burnished magnesium alloy

    Directory of Open Access Journals (Sweden)

    Zaleski Radosław

    2015-12-01

    Full Text Available The effect of roller burnishing on Vickers’ hardness and positron lifetimes in the AZ91HP magnesium alloy was studied. The microhardness increases with an increase in the burnishing force and with a decrease in the feed. The comparison of various methods of analysis of positron annihilation lifetime (PAL spectra allowed identification of two components, which are related to solute-vacancy complexes and vacancy clusters, respectively. It was found that the increase in microhardness was related to the increase in the concentration of vacancy clusters.

  16. Absorbed dose in polymers during a positron annihilation experiment

    International Nuclear Information System (INIS)

    Suzuki, T.; Namito, Y.; Oki, Y.; Numajiri, M.; Miura, T.; Hirayama, H.; Kondo, K.; Ito, Y.

    1994-01-01

    A positron annihilation lifetime (PAL) technique has been recognized as being a useful method to study the characteristics of polymers. However, radiation effects due to positrons used as a probe have been raised as being a problem, since positrons emitted from 22 Na have sufficient energy to induce radiation damage in polymers. In this study, the radiation dose induced by positrons emitted from 22 Na was estimated for such polymers like polyethylenes and polypropylenes using the EGS4 code. The radiation damage during PAL measurements is also discussed. It has been shown that the calculated dose is consistent with that estimated from an empirical equation of the mass-attenuation coefficient. (author)

  17. Morphology of Thermoset Polyimides by Positron Annihilation Spectroscopy

    Science.gov (United States)

    Ranganathaiah, C.; Pater, R. H.; Sprinkle, D. R.; Baugher, A. H.; Eftekhari, A.; Singh, J. J.

    1994-01-01

    Thermoset polyimides have great potential for successfully meeting tough stress and temperature challenges in the advanced aircraft development program. However, studies of structure/property relationships in these materials have not been very successful so far. Positron annihilation spectroscopy has been used to investigate free volumes and associated parameters. It has been noted that the free volume correlates well with the molecular weight, cross-link density and thermal coefficient of expansion of these materials. Currently no other techniques are available for direct measurement of these parameters. Experimental results and their interpretations will be discussed.

  18. Fatigue damage in superalloys determined using Doppler broadening positron annihilation

    Science.gov (United States)

    Hoeckelman, Donald; Leighly, H. P., Jr.

    1990-01-01

    Axial fatigue specimens of three superalloys, Inconel 718, Incoloy 903 and Haynes 188, were machined from solution-heat-treated material and artificially aged. They were subjected to cyclic loading for a selected number of cycles after which the S parameter was determined using Doppler broadening positron annihilation. Initially, the S parameter decreased, followed by a large increase and a subsequent decline leading to fracture. This has been interpreted as the removal of residual vacancies, the introduction of new defects by cyclic loading, and, finally, a clustering of the defects as microcracks which grow to cause failure.

  19. The wish for annihilation in 'love-death' as collapse of the need for recognition, in Wagner's Tristan und Isolde.

    Science.gov (United States)

    Bergstein, Moshe

    2013-08-01

    Wagner's Tristan und Isolde holds a central position in Western music and culture. It is shown to demonstrate consequences of interruption of developmental processes involving the need for recognition of subjectivity, resulting in the collapse of this need into the wish for annihilation of self and other through 'love-death' [Liebestod]. A close reading of the musical language of the opera reveals how this interruption is demonstrated, and the consequent location of identity outside of language, particularly suitable for expression in music. Isolde's dynamics are presented as distinct from that of Tristan, and in contrast to other interpretations of Tristan and Isolde's love as an attack on the Oedipal order, or as a regressive wish for pre-Oedipal union. Isolde's Act I narrative locates the origin of her desire in the protagonists' mutual gaze at a traumatic moment. In this moment powerful and contrasting emotions converge, evoking thwarted developmental needs, and arousing the fantasy of redemption in love-death. By removing the magical elements, Wagner enables a deeper understanding of the characters' positions in relation to each other, each with his or her own needs for recognition and traumatic experiences. These positions invite mutual identifications resulting in rising tension between affirmation of identity and annihilation, with actual death as the only possible psychic solution. The dynamics described in the opera demonstrate the function of music and opera in conveying meaning which is not verbally expressible. Copyright © 2013 Institute of Psychoanalysis.

  20. New insights into the nanostructure of innovative thin film solar cells gained by positron annihilation spectroscopy

    NARCIS (Netherlands)

    Eijt, S.W.H.; Shi, W.; Mannheim, A.; Butterling, M.; Schut, H.; Egger, W; Dickmann, M.; Hugenschmidt, C; Shakeri, B.; Meulenberg, R; Callewaert, V.; Saniz, R; Partoens, B; Barbiellini, B; Bansil, A; Melskens, J.; Zeman, M.; Smets, A.H.M.; Kulbak, M.; Hodes, G.; Cahen, D.; Brück, E.H.

    2017-01-01

    Recent studies showed that positron annihilation methods can provide key insights into the nanostructure and electronic structure of thin film solar cells. In this study, positron annihilation lifetime spectroscopy (PALS) is applied to investigate CdSe quantum dot (QD) light absorbing layers,

  1. CMB bounds on dark matter annihilation: Nucleon energy losses after recombination

    NARCIS (Netherlands)

    Weniger, C.; Serpico, P.D.; Iocco, F.; Bertone, G.

    2013-01-01

    We consider the propagation and energy losses of protons and antiprotons produced by dark matter annihilation at redshifts 100annihilations into quarks, gluons and weak gauge bosons, protons and antiprotons carry about 20% of the energy injected into e± and γ’s,

  2. Bounds on Dark Matter annihilations from 21 cm data arXiv

    CERN Document Server

    D'Amico, Guido; Strumia, Alessandro

    The observation of an absorption feature in the 21 cm spectrum at redshift $z\\approx 17$ implies bounds on Dark Matter annihilations for a broad range of masses, given that significant heating of the intergalactic medium would have erased such feature. The resulting bounds on the DM annihilation cross sections are comparable to the strongest ones from all other observables.

  3. How to distinguish between the annihilation and the creation of optical vortices.

    Science.gov (United States)

    Roux, Filippus S

    2013-10-01

    Optical vortices are always created or annihilated as vortex dipoles-pairs with opposite topological charge. Here a quantity, consisting of the transverse first and second derivatives of the optical field, is derived with which one can distinguish between vortex dipole annihilation and creation events. Analytical and numerical examples are provided as a demonstration of the method.

  4. Positron annihilation in disordered regions in neutron-irradiated Ge and Si

    International Nuclear Information System (INIS)

    Pustovoit, A.K.; Konopleva, R.F.; Kupchishin, A.I.; Mukashev, K.M.

    1989-01-01

    The method of angular distribution of annihilation photons was used to investigate the formation and annealing of radiation defects in Ge and Si irradiated with reactor neutrons. These effects were studied as a function of the type of conduction of the dopant concentration. The nature of annealing demonstrated positron annihilation at multivacancy complexes located within disordered regions

  5. An Experiment to Demonstrate the Energy Broadening of Annihilation Gamma Rays

    Science.gov (United States)

    Ouseph, P. J.; DuBard, James L.

    1978-01-01

    Shows that when positions annihilate in solid materials the energy distribution of the annihilation gamma rays is much broader than that of a 0.511-Mev gamma peak. This broadening is caused by the momentum distribution of the electrons in the material. (Author/GA)

  6. A Position Annihilation Study of Defect Recovery in Electron-Irradiated alpha-Zr

    DEFF Research Database (Denmark)

    Hood, G. M.; Eldrup, Morten Mostgaard; Mogensen, O. E.

    1977-01-01

    The presence of vacancy defects in α-Zr, irradiated at 320 > T > 290 K with 1.5 MeV electrons, has been indicated by positron annihilation measurements. It was found that positron lifetimes associated with annihilation in well-annealed α-Zr, fell in the range 173 to 181 psec, with no obvious...

  7. Antiproton annihilation physics annihilation physics in the Monte Carlo particle transport code particle transport code SHIELD-HIT12A

    DEFF Research Database (Denmark)

    Taasti, Vicki Trier; Knudsen, Helge; Holzscheiter, Michael

    2015-01-01

    –Teller Z-law, which is implemented by default in SHIELD-HIT12A has been shown not to be a good approximation for the capture probability of negative projectiles by nuclei. We investigate other theories which have been developed, and give a better agreement with experimental findings. The consequence...... sections, which restores the agreement, but some small deviations still remain. Best agreement is achieved by using the most recent antiproton collision cross sections and the Fermi–Teller Z-law, even if experimental data conclude that the Z-law is inadequately describing annihilation on compounds. We...

  8. Proposed method to construct Boolean functions with maximum possible annihilator immunity

    Science.gov (United States)

    Goyal, Rajni; Panigrahi, Anupama; Bansal, Rohit

    2017-07-01

    Nonlinearity and Algebraic(annihilator) immunity are two core properties of a Boolean function because optimum values of Annihilator Immunity and nonlinearity are required to resist fast algebraic attack and differential cryptanalysis respectively. For a secure cypher system, Boolean function(S-Boxes) should resist maximum number of attacks. It is possible if a Boolean function has optimal trade-off among its properties. Before constructing Boolean functions, we fixed the criteria of our constructions based on its properties. In present work, our construction is based on annihilator immunity and nonlinearity. While keeping above facts in mind,, we have developed a multi-objective evolutionary approach based on NSGA-II and got the optimum value of annihilator immunity with good bound of nonlinearity. We have constructed balanced Boolean functions having the best trade-off among balancedness, Annihilator immunity and nonlinearity for 5, 6 and 7 variables by the proposed method.

  9. Characterization of the melting process of PTFE using positron annihilation spectroscopy

    International Nuclear Information System (INIS)

    Honda, Y; Nishijima, S

    2015-01-01

    Poly(tetrafluoroethylene) (PTFE) is a semi-crystalline polymer and the lifetime of ortho-positronium(o-Ps) is known to be able to be separated into two components due to annihilation in the crystal region and in the amorphous region. The melting process of PTFE was investigated using positron annihilation spectroscopy and X-ray diffraction. The results indicated that volume expansion with an increase of temperature is dominantly due to the expansion of the amorphous region and a Ps bubble is formed at melting in both regions. The o-Ps relating to the crystal region definitely remains on the surface of crystal at the time of annihilation. The production of lower energy electrons at melting was deduced by the analysis of the Doppler broadened annihilation photopeak, and the increase in the number of such electrons was found to have great influence on the formation of the o-Ps and annihilation processes of positron and o-Ps. (paper)

  10. Positron annihilation in modified zeolites LTA and 13X

    Energy Technology Data Exchange (ETDEWEB)

    Cabral-Prieto, A.; Garcia-Sosa, I.; Jimenez-Becerril, J. [Departamento de Quimica, Instituto Nacional de Investigaciones Nucleares, Apartado Postal 18-1027, Col. Escandon, Del. M. Hidalgo, Mexico D. F., c. p. 11801 (Mexico); Lopez-Castanares, R.; Olea-Cardoso, O. [Facultad de Quimica, Universidad Autonoma del Estado de Mexico, Paseo Tollocan esquina paseo Tollocan, esquina paseo Colon, Toluca, c. p. 50120, Estado de Mexico (Mexico)

    2007-07-01

    The pick-off annihilation lifetimes of o -Ps, {tau}{sub po}, in dehydrated Co{sup 2+} and Mn{sup 2+} exchanged zeolites LTA, in dehydrated Co{sup 2+} exchanged zeolite 13X, and in dehydrated Na{sup +} zeolites LTA and 13X, are estimated. Although {tau}{sub po} can be estimated from the lifetime spectra of the cation exchanged zeolites LTA and 13X, this lifetime can not be estimated from those spectra of Na{sup +} zeolite LTA unambiguously. The estimated pick-off lifetimes due to the annihilation of o-Ps in the internal walls of the zeolites are systematically lower than the average lifetime of p-Ps and o-Ps in vacuum {tau}{sub a}=0.5 ns. Since the pick-off process of o-Ps occurs particularly on the internal cavity walls of dehydrated zeolites, the replacement of {tau}{sub a} by {tau}{sub po} within the classical model of Tao-Eldrup to calculate cavity radius should provide more realistic cavity radii of these porous materials than when using {l_brace}{tau}{sub a}{r_brace}. This suggestion is supported by previous and present results. (copyright 2007 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

  11. Extinction and survival in two-species annihilation

    Science.gov (United States)

    Amar, J. G.; Ben-Naim, E.; Davis, S. M.; Krapivsky, P. L.

    2018-02-01

    We study diffusion-controlled two-species annihilation with a finite number of particles. In this stochastic process, particles move diffusively, and when two particles of opposite type come into contact, the two annihilate. We focus on the behavior in three spatial dimensions and for initial conditions where particles are confined to a compact domain. Generally, one species outnumbers the other, and we find that the difference between the number of majority and minority species, which is a conserved quantity, controls the behavior. When the number difference exceeds a critical value, the minority becomes extinct and a finite number of majority particles survive, while below this critical difference, a finite number of particles of both species survive. The critical difference Δc grows algebraically with the total initial number of particles N , and when N ≫1 , the critical difference scales as Δc˜N1 /3 . Furthermore, when the initial concentrations of the two species are equal, the average number of surviving majority and minority particles, M+ and M-, exhibit two distinct scaling behaviors, M+˜N1 /2 and M-˜N1 /6 . In contrast, when the initial populations are equal, these two quantities are comparable M+˜M-˜N1 /3 .

  12. Leptons from Dark Matter Annihilation in Milky Way Subhalos

    CERN Document Server

    Cline, James M; Xue, Wei

    2010-01-01

    Numerical simulations of dark matter collapse and structure formation show that in addition to a large halo surrounding the baryonic component of our galaxy, there also exists a significant number of subhalos that extend hundreds of kiloparsecs beyond the edge of the observable Milky Way. We find that for dark matter (DM) annihilation models, galactic subhalos can significantly modify the spectrum of electrons and positrons as measured at our galactic position. Using data from the recent Via Lactea II simulation we include the subhalo contribution of electrons and positrons as boundary source terms for simulations of high energy cosmic ray propagation with a modified version of the publicly available GALPROP code. Focusing on the DM DM -> 4e annihilation channel, we show that including subhalos leads to a better fit to both the Fermi and PAMELA data. The best fit gives a dark matter particle mass of 1.2 TeV, for boost factors of 90 in the main halo and 1950-3800 in the subhalos (depending on assumptions about...

  13. Positron annihilation in polymers and permeability of gases

    International Nuclear Information System (INIS)

    Buriova, E.

    2001-05-01

    An analysis of positron annihilation spectroscopy (PAS) results for different substituted polyacetylenes samples under vacuum and in air is presented with the aim to investigate the influence of the external atmosphere on the experimental PAS measurements and to determine correctly the size and the number of the free volume holes. The existence of special structure elements in polymers is responsible for the appearance of the fourth component of the time spectrum. The latter is formed at the expense of free volume elements in disordered regions of the polymer. A study of a number of glassy polymers with widely varying free volume and gas permeability showed that a bimodal size distribution of free volume elements is not an exception in some polymers but is a typical feature of the microstructure of amorphous glassy polymers. Oxygen-induced quenching of positronium lifetimes is demonstrated for all polymer samples. Good correlation of permeability of polymers with the size of free volume elements is demonstrated. This correlation can be used for a fast assessment of gas permeation properties of novel polymers using positron annihilation data (author)

  14. Relative Biological Effectiveness and Peripheral Damage of Antiproton Annihilation

    CERN Multimedia

    Kavanagh, J N; Kaiser, F; Tegami, S; Schettino, G; Kovacevic, S; Hajdukovic, D; Knudsen, H; Currell, F J; Toelli, H T; Doser, M; Holzscheiter, M; Herrmann, R; Timson, D J; Alsner, J; Landua, R; Comor, J; Moller, S P; Beyer, G

    2002-01-01

    The use of ions to deliver radiation to a body for therapeutic purposes has the potential to be significant improvement over the use of low linear energy transfer (LET) radiation because of the improved energy deposition profile and the enhanced biological effects of ions relative to photons. Proton therapy centers exist and are being used to treat patients. In addition, the initial use of heavy ions such as carbon is promising to the point that new treatment facilities are planned. Just as with protons or heavy ions, antiprotons can be used to deliver radiation to the body in a controlled way; however antiprotons will exhibit additional energy deposition due to annihilation of the antiprotons within the body. The slowing down of antiprotons in matter is similar to that of protons except at the very end of the range beyond the Bragg peak. Gray and Kalogeropoulos estimated the additional energy deposited by heavy nuclear fragments within a few millimeters of the annihilation vertex to be approximately 30 MeV (...

  15. Calculating the annihilation rate of weakly interacting massive particles.

    Science.gov (United States)

    Baumgart, Matthew; Rothstein, Ira Z; Vaidya, Varun

    2015-05-29

    We develop a formalism that allows one to systematically calculate the weakly interacting massive particle (WIMP) annihilation rate into gamma rays whose energy far exceeds the weak scale. A factorization theorem is presented which separates the radiative corrections stemming from initial-state potential interactions from loops involving the final state. This separation allows us to go beyond the fixed order calculation, which is polluted by large infrared logarithms. For the case of Majorana WIMPs transforming in the adjoint representation of SU(2), we present the result for the resummed rate at leading double-log accuracy in terms of two initial-state partial-wave matrix elements and one hard matching coefficient. For a given model, one may calculate the cross section by finding the tree level matching coefficient and determining the value of a local four-fermion operator. The effects of resummation can be as large as 100% for a 20 TeV WIMP. However, for lighter WIMP masses relevant for the thermal relic scenario, leading-log resummation modifies the Sudakov factors only at the 10% level. Furthermore, given comparably sized Sommerfeld factors, the total effect of radiative corrections on the semi-inclusive photon annihilation rate is found to be percent level. The generalization of the formalism to other types of WIMPs is discussed.

  16. Zadig: latest improvements to Bremsstrahlung treatment and in-flight annihilation scheme

    International Nuclear Information System (INIS)

    Menard, St.

    2006-01-01

    Multigroup cross-section for the 3-dimensional Monte-Carlo transport code DIANE are produced by the ZADIG code. Although DIANE does not transport the electrons and positrons, the production of Bremsstrahlung photons induced by the electrons and positrons during their slowing down is taken into account in the ZADIG code because the electron-gamma cascade is an important process in high energy gamma ray transport. ZADIG does not distinguish positrons from electrons except for the positron annihilation. However, the user can turn on this direction. This report presents the latest improvements to the Bremsstrahlung model of ZADIG and to the positron annihilation algorithm implemented in the code. Positrons can annihilate either in flight or at rest in the latest release of ZADIG. As MCNP does not take into account the annihilation in flight, results of ZADIG-DIANE calculations are compared to the results of GEANT-4 in order to validate the annihilation scheme of ZADIG. The results with annihilation divided by the results without present similar trends between 0.6 and 10 MeV for the 2 codes (GEANT-4 and ZADIG-DIANE), in other words an influence of 5%, so the annihilation scheme programmed in ZADIG appears to be satisfying and can be considered as validated

  17. Positron annihilation characterization of Fe-Y2O3 composite powder after mechanical alloying and heat treatment.

    Science.gov (United States)

    Lee, Jae Hoon

    2012-02-01

    Fe-1 wt% Y2O3 composite powders were mechanically alloyed for 12 hr and then heat-treated at 1050 degrees C for 1 hr. Positron annihilation lifetime and coincidence Doppler broadening measurements are in qualitative agreement with X-ray diffraction studies, indicating that in the as-mixed Fe-1Y2O3 composite, up to approximately equal to 70% of the annihilations occur at vacancy clusters; a small fraction annihilates in its matrix. In the case of mechanically alloyed composite, up to approximately equal to 60% of the positrons annihilate at vacancy clusters. Some annihilations also occur in dislocations. In the heat-treated Fe-1Y2O3, positrons primarily annihilate at yttria precipitates, while a small fraction annihilates in the matrix.

  18. Higgs shifts from electron-positron annihilations near neutron stars

    Energy Technology Data Exchange (ETDEWEB)

    Wegner, Gary A. [Dartmouth College, Department of Physics and Astronomy, Hanover, NH (United States); Onofrio, Roberto [Universita di Padova, Dipartimento di Fisica e Astronomia ' Galileo Galilei' , Padova (Italy); ITAMP, Harvard-Smithsonian Center for Astrophysics, Cambridge, MA (United States)

    2015-07-15

    We discuss the potential for using neutron stars to determine bounds on the Higgs-Kretschmann coupling by looking at peculiar shifts in gamma-ray spectroscopic features. In particular, we reanalyze multiple lines observed in GRB781119 detected by two gamma-ray spectrometers, and derive an upper bound on the Higgs-Kretschmann coupling that is much more constraining than the one recently obtained from white dwarfs. This calls for targeted analyses of spectra of gamma-ray bursts from more recent observatories, dedicated searches for differential shifts on electron-positron and proton-antiproton annihilation spectra in proximity of compact sources, and signals of electron and proton cyclotron lines from the same neutron star. (orig.)

  19. Angular correlation of annihilation photons in ice single crystals

    DEFF Research Database (Denmark)

    Mogensen, O. E.; Kvajic, G.; Eldrup, Morten Mostgaard

    1971-01-01

    -lattice vectors g⃗ on the direction perpendicular to the slits and the sample surface. The relative area of the central plus the side peaks was (15.2 ± 0.4)% for all curves. All the peaks are interpreted as due to parapositronium annihilation. The side peaks are explained as evidence for the positronium center......Linear-slit angular-correlation curves were obtained at - 148 °C for the [0001], [10¯10], and [11¯20] directions in single crystals of ice. Besides the narrow central peak, pronounced narrow side peaks were also observed. They occurred at angles θ=2πℏgz/mc, where gz is the projection of reciprocal...

  20. Gamma and pizero production in e+e- annihilation

    International Nuclear Information System (INIS)

    Fong, A.

    1980-01-01

    Inclusive cross sections of γ's and π 0 mesons in hadronic events produced by electron-positron annihilation for the center-of-mass energy range 4.9 to 7.4 GeV are presented. Scale invariance of the inclusive spectra is exhibited in this energy range, and their normalization and shape are seen to be consistent with those of spectra arising from the decay of the π 0 . The fraction of center-of-mass energy carried away by the γ's at high energies is found to be = 0.24 +- 0.01. The π 0 inclusive cross section is seen to be consistent in normalization and shape with half the charged-π cross section between x = 0.15 and 0.75, with an integrated inclusive cross-section ratio of sigma(π 0 )/[sigma(π + ) + sigma(π - )] = 0.48 +- 0.05. 60 figures, 7 tables

  1. Electronic Structure of Rare-Earth Metals. II. Positron Annihilation

    DEFF Research Database (Denmark)

    Williams, R. W.; Mackintosh, Allan

    1968-01-01

    The angular correlation of the photons emitted when positrons annihilate with electrons has been studied in single crystals of the rare-earth metals Y, Gd, Tb, Dy, Ho, and Er, and in a single crystal of an equiatomic alloy of Ho and Er. A comparison of the results for Y with the calculations...... of Loucks shows that the independent-particle model gives a good first approximation to the angular distribution, although correlation effects probably smear out some of the structure. The angular distributions from the heavy rare-earth metals are very similar to that from Y and can be understood...... qualitatively in terms of the relativistic augmented-plane-wave calculations by Keeton and Loucks. The angular distributions in the c direction in the paramagnetic phases are characterized by a rapid drop at low angles followed by a hump, and these features are associated with rather flat regions of Fermi...

  2. Positron annihilation in hydrogenated and electron-irradiated titanium alloys

    International Nuclear Information System (INIS)

    Mukashev, K.M.; Zaikin, Yu.A.

    2002-01-01

    Important information on hydrogen behavior in titanium can be obtained from studies of radiation damage in previously hydrogenated metal. For this purpose annealed titanium samples were hydrogenated at the temperature 500 deg. C during 1 hour. Then both the original annealed samples and hydrogenated samples were irradiated by 4 MeV electrons in the fluence range 3·10 7 -1·10 19 cm - 2 at the temperature 60 deg. C. It is known that electron irradiation in these conditions predominantly creates vacancy-type defects with an average radius R ν =0.81 Angstrom. It was stated that annihilation probability after electron irradiation of previously hydrogenated titanium samples always has some intermediate values between those characteristic for hydrogenated and irradiated states of previously annealed metal. This is a reason to suppose that radiation defects of the vacancy type in previously hydrogenated titanium combine with hydrogen atoms in favorable conditions of their partial ionization. The estimated value of the average radius for such a complex is R ν =1.1 Angstrom, that is higher than vacancy size but lower than an atom radius. No dose dependence of hydrogen interaction with radiation defects was observed in our experiments.The results of isochrone annealing of the materials under study have shown that the single annealing recovery stage with activation energy E a equal to 1.22 eV is observed in electron irradiated but not previously hydrogenated titanium in the temperature range 170-240 deg. C. Electron irradiation of the previously hydrogenated metal shifts beginning of the first recovery stage to the temperature about 225-230 deg. C and finishes near the temperature 330 deg. C. Therefore, the bound state vacancy-hydrogen in titanium is characterized by higher temperature range of dissociation and annealing with activation energy equal to 1.38 eV. However, subsequent measurements, of the angular distribution of annihilation photons (ADAP) have demonstrated

  3. Spiral Calcium Wave Propagation and Annihilation in Xenopus laevis Oocytes

    Science.gov (United States)

    Lechleiter, James; Girard, Steven; Peralta, Ernest; Clapham, David

    1991-04-01

    Intracellular calcium (Ca2+) is a ubiquitous second messenger. Information is encoded in the magnitude, frequency, and spatial organization of changes in the concentration of cytosolic free Ca2+. Regenerative spiral waves of release of free Ca2+ were observed by confocal microscopy in Xenopus laevis oocytes expressing muscarinic acetylcholine receptor subtypes. This pattern of Ca2+ activity is characteristic of an intracellular milieu that behaves as a regenerative excitable medium. The minimal critical radius for propagation of focal Ca2+ waves (10.4 micrometers) and the effective diffusion constant for the excitation signal (2.3 x 10-6 square centimeters per second) were estimated from measurements of velocity and curvature of circular wavefronts expanding from foci. By modeling Ca2+ release with cellular automata, the absolute refractory period for Ca2+ stores (4.7 seconds) was determined. Other phenomena expected of an excitable medium, such as wave propagation of undiminished amplitude and annihilation of colliding wavefronts, were observed.

  4. A multi-parameter, acquisition system positron annihilation lifetime spectrometer

    International Nuclear Information System (INIS)

    Sharshar, T.

    2004-01-01

    A positron annihilation lifetime spectrometer employing a multi-parameter acquisition system has been prepared for various purposes such as the investigation and characterization of solid-state materials. The fast-fast coincidence technique was used in the present spectrometer with a pair of plastic scintillation detectors. The acquisition system is based on the Kmax software and on CAMAC modules. The data are acquired in event-by-event list mode. The time spectrum for the desired energy windows can be obtained by off-line data sorting and analysis. The spectrometer for event-by-event data acquisition is an important step to construct a positron age-momentum correlation (AMOC) spectrometer. The AMOC technique is especially suited for the observation of positron transitions between different states during their lifetime. The system performance was tested and the results were presented and discussed

  5. Development of positron annihilation spectroscopy for characterizing neutron irradiated tungsten

    Energy Technology Data Exchange (ETDEWEB)

    C.N. Taylor; M. Shimada; D.W. Akers; M.W. Drigert; B.J. Merrill; Y. Hatano

    2013-05-01

    Tungsten samples (6 mm diameter, 0.2 mm thick) were irradiated to 0.025 and 0.3 dpa with neutrons in the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory. Samples were then exposed to deuterium plasma in the tritium plasma experiment (TPE) at 100, 200 and 500ºC to a total fluence of 1 x 1026 m-2. Nuclear reaction analysis (NRA) and Doppler broadening positron annihilation spectroscopy (DB-PAS) were performed at various stages to characterize damage and retention. We present the first known results of neutron damaged tungsten characterized by DB-PAS in order to study defect concentration. Two positron sources, 22Na and 68Ge, probe ~58 µm and through the entire 200 µm thick samples, respectively. DB-PAS results reveal clear differences between the various irradiated samples. These results, and the calibration of DB-PAS to NRA data are presented.

  6. Moisture dependence of positron annihilation spectra in nylon-6

    Science.gov (United States)

    Singh, J. J.; St. Clair, T. L.; Holt, W. H.; Mock, W., Jr.

    1984-01-01

    Positron annihilation time spectra have been measured in nylon-6 samples as a function of their moisture content. The measured average long life component lifetime values are: 1722 + or - 47 ps (dry), 1676 + or - 40 ps (14.6 percent saturation value), 1719 + or - 26 ps (29.3 percent saturation value), 1720 + or - 35 ps (50 percent of saturation value), 1857 + or - 35 ps (78.1 percent saturation value), and 1936 + or - 57 ps (saturated). It appears that nylon-6 has a special affinity for water at low concentration levels where H2O molecules enter between the (C = O - H-N) chemical bonds between nylon molecular chains. As the water concentration increases beyond a critical level, nylon-6 specimens start trapping H2O molecules in other bond sites or potential wells. The trapped water increases the free volume in the test specimens and reduces Ps atom formation as well as its subsequent decay rate.

  7. Study of ion beam induced depolymerization using positron annihilation techniques

    Energy Technology Data Exchange (ETDEWEB)

    Puglisi, O. E-mail: opuglisi@dipchi.unict.it; Fragala, M.E.; Lynn, K.G.; Petkov, M.; Weber, M.; Somoza, A.; Dupasquier, A.; Quasso, F

    2001-04-01

    Ion beam induced depolymerization of polymers is a special class of ion beam induced chemical reaction which gives rise to catastrophic 'unzipping' of macromolecules with production of large amounts of the monomer, of the order of many hundreds monomer molecules per each macromolecule. The possible modification of the density at microscopic level prompted us to undertake a study of this effect utilizing positron annihilation techniques in Poly(methylmethacrylate) (PMMA) before and after bombardment with He{sup +} 300 keV ions at 200 deg. C. Preliminary results shown here indicate that before bombardment there is a reproducible dependence of nano-hole distribution on the sample history. Moreover at 200 deg. C we do not detect formation of new cavities as a consequence of the strong depolymerization that occurs under the ion beam. The possible correlation of these findings with transport properties of PMMA at temperature higher than the glass transition temperature will be discussed.

  8. Positron annihilation studies of vacancies in Ag-Zn alloys

    International Nuclear Information System (INIS)

    Chabik, S.

    1982-01-01

    The temperature dependence of annihilation rate, F(T), at the peak of angular correlation curve has been measured for Ag-29.2%at Zn and Ag-50%at Zn alloys. By applying the trapping model the vacancy formation energy for Ag-29.2%at Zn alloy has been found to be equal to 0.94+-0.06 eV. It has been found that the course of the F(T) curve for Ag-50%at Zn depends on the phase composition and thermal history of the investigated sample. For alloys containing not more than 50%at Zn, the concentration dependence of the vacancy formation energy for Ag-Zn alloys is very similar to that for Cu-Zn alloys. (Auth.)

  9. Work station for low temperature positron annihilation studies

    International Nuclear Information System (INIS)

    Chaturvedi, T.P.; Venkiteswaran, S.; Pujari, P.K.

    1999-05-01

    This report describes the automation implemented in the low temperature Positron Annihilation Spectroscopy studies system. Temperature programmer and controller (Lakeshore 330) is interfaced to PC-AT through an IEEE-488 add-on card. Through this data can be read and written to the temperature controller and it can be handled remotely. The PC- AT also houses the PCA-II card. Software (TEMP330.EXE) was developed to communicate with the temperature controller. A master software is also developed under which TEMP330.EXE and PCAII.EXE should run. Another program DATASEG.EXE creates a user file to store the temperature points given by user over which data acquisition is required. This has not only widened the scope of the positron research, but also helps achieve result with better precision. (author)

  10. Positron annihilation studies on reactor irradiated and thermal annealed ferrocene

    International Nuclear Information System (INIS)

    Marques Netto, A.; Carvalho, R.S.; Magalhaes, W.F.; Sinisterra, R.D.

    1996-01-01

    Retention and thermal annealing following (n, γ) reaction in solid ferrocene, Fe(C 5 H 5 ) 2 , were studied by positron annihilation lifetime spectroscopy (PAL). Positronium (Ps) formation was observed in the non-irradiated compound with a probability or intensity (I 3 ) of 30%. Upon irradiation of the compound with thermal neutrons in a nuclear reactor, I 3 decreases with increasing irradiation time. Thermal treatment again increases I 3 values from 16% to 25%, revealing an important proportion of molecular reformation without variation of the ortho-positronium lifetime (τ 3 ). These results point out the major influence of the electronic structure as determining the Ps yields in the pure complex. In the irradiated and non irradiated complexes the results are satisfactorily explained on the basis of the spur model. (orig.)

  11. An observation of annihilation radiation from the Galactic center region

    Science.gov (United States)

    Matteson, J.; Pelling, M.; Peterson, L.; Bowman, B.; Briggs, M.; Lingenfelter, R.; Lin, R.; Smith, D.; Feffer, P.; Pehl, R.

    1991-01-01

    Results are reported from observations of the 511 MeV annihilation gamma-ray line from the Galactic center, made on May 22, 1989 with a high-resolution gamma-ray spectrometer on board a balloon launched from Alice Springs (Australia). The observations were made at about 4 gm/sq cm atmospheric depth for 6 hrs in a series of target and background pointings lasting 20 min each. The results obtained from multiparameter Gaussian fits to the data were as follows: 511 keV flux = 0.00089 + or - 0.00027 ph/sq cm per sec-rad, line width of about 1.1 keV, and less than 3.2 keV FWHM at 95 percent confidence.

  12. Probing Positron Cooling in Noble Gases via Annihilation γ Spectra.

    Science.gov (United States)

    Green, D G

    2017-11-17

    γ spectra for positron annihilation in noble-gas atoms are calculated using many-body theory for positron momenta up to the positronium-formation threshold. These data are used, together with time-evolving positron-momentum distributions determined in the preceding Letter [Phys. Rev. Lett. 119, 203403 (2017)PRLTAO0031-9007], to calculate the time-varying γ spectra produced during positron cooling in noble gases. The γ spectra and their S[over ¯] and W[over ¯] shape parameters are shown to be sensitive probes of the time evolution of the positron momentum distribution and thus provide a means of studying positron cooling that is complementary to positron lifetime spectroscopy.

  13. Dark matter annihilation through a lepton-specific Higgs boson

    Science.gov (United States)

    Logan, Heather E.

    2011-02-01

    It was recently argued by Hooper and Goodenough [arXiv:1010.2752] that the excess gamma-ray emission from within 1°-2° of the Galactic center can be well described by annihilation of ˜8GeV dark matter particles into tau pairs. I show that such a dark matter signal can be obtained naturally in the lepton-specific two-Higgs-doublet model extended by a stable singlet scalar dark matter candidate. The favored parameter region prefers a light Higgs state (below 200 GeV) with enhanced couplings to leptons and a sizable invisible branching fraction. Part of the favored region leads to invisible decays of both of the CP-even neutral Higgs states.

  14. Antiprotons from dark matter annihilation in the Galaxy. Astrophysical uncertainties

    Energy Technology Data Exchange (ETDEWEB)

    Evoli, Carmelo [Chinese Academy of Sciences, Beijing (China). National Astronomical Observatories; Cholis, Ilias; Ullio, Piero [SISSA, Sezione di Trieste (Italy); INFN, Sezione di Trieste (Italy); Grasso, Dario [INFN, Sezione di Pisa (Italy); Maccione, Luca [Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)

    2011-08-15

    The latest years have seen steady progresses in WIMP dark matter (DM) searches, with hints of possible signals suggested by both direct and indirect detection experiments. Antiprotons can play a key role validating those interpretations since they are copiously produced by WIMP annihilations in the Galactic halo, and the secondary antiproton background produced by Cosmic Ray (CR) interactions is predicted with fair accuracy and matches the observed spectrum very well. Using the publicly available numerical DRAGON code, we reconsider antiprotons as a tool to constrain DM models discussing its power and limitations. We provide updated constraints on a wide class of annihilating DM models by comparing our predictions against the most up-to-date anti p measurements, taking also into account the latest spectral information on the p, He and other CR nuclei fluxes. Doing that, we probe carefully the uncertainties associated to both secondary and DM originated antiprotons, by using a variety of distinctively different assumptions for the propagation of CRs and for the DM distribution in the Galaxy. We find that the impact of the astrophysical uncertainties on constraining the DM properties can be much stronger, up to a factor of {proportional_to}50, than the one due to uncertainties on the DM distribution ({proportional_to}2-6). Remarkably, even reducing the uncertainties on the propagation parameters derived by local observables, non-local effects can still change DM model constraints even by 50%. Nevertheless, current anti p data place tight constraints on DM models, excluding some of those suggested in connection with indirect and direct searches. Finally we discuss the power of upcoming CR spectral data from the AMS-02 observatory to drastically reduce the uncertainties discussed in this paper and estimate the expected sensitivity of this instrument to some sets of DM models. (orig.)

  15. OSSE observations of galactic 511 keV annihilation radiation

    Science.gov (United States)

    Purcell, W. R.; Grabelsky, D. A.; Johnson, W. N.; Jung, G. V.; Kinzer, R. L.; Kurfess, J. D.; Strickman, M. S.; Ulmer, M. P.

    1992-01-01

    The Oriented Scintillation Spectrometer Experiment (OSSE) on the Compton Gamma-Ray Observatory has performed several observations of the galactic plane and galactic center region to measure the distribution of galactic 511 keV positron annihilation radiation. Preliminary analysis of data collected during the observation of the galactic center region over the period 13-24 Jun. 1991, indicates the presence of a 511 keV line and positronium continuum superimposed on a power-law continuum. The line of flux was found to be (2.7 +/- 0.5) x 10(exp -4) gamma/sq cm sec, with a positronium fraction of (0.9 +/- 0.2). The 3(sigma) upper limit to daily variations in the 511 keV line flux from the mean during the observation interval is 3 x 10(exp -4) gamma/sq cm sec. If all of the observed annihilation radiation is assumed to originate from the x-ray source 1E 1740.7-2942, the corresponding 511 keV line flux would be (3.0 +/- 0.6) x 10(exp -4) gamma/sq cm sec. The 3(sigma) upper limit for 511 keV line emission from the x-ray binary GX1+4 is 6 x 10(exp -4) gamma/sq cm sec. Results from the galactic plane observations at galactic longitudes of 25 degrees (16-21 Aug. 1991) and 339 degrees (6-11 Sep. 1991) suggest that the emission is concentrated near the galactic center. The observations and the preliminary results are described.

  16. Concept and viability of androgen annihilation for advanced prostate cancer.

    Science.gov (United States)

    Mohler, James L

    2014-09-01

    There remains no standard of care for patients with a rising prostate-specific antigen level after radical prostatectomy or radiotherapy but who have no radiographic metastases, even though this is the second largest group of patients with prostate cancer (CaP) in the United States. Androgen deprivation therapy (ADT) may cure some men with advanced CaP based on single-institution series and a randomized clinical trial of immediate versus delayed ADT for men found to have pelvic lymph node metastasis at the time of radical prostatectomy. ADT may be more effective when initiated for minimal disease burden, which can be detected using PSA after radical prostatectomy or radiotherapy, and if more complete disruption of the androgen axis using newer agents decreases the chance that androgen-sensitive cells survive to adapt to a low-androgen environment. Androgens may be "annihilated" simultaneously using a luteinizing hormone-releasing hormone antagonist or agonist to inhibit testicular production of testosterone, a P45017A1 (CYP17A1) inhibitor to diminish metabolism of testosterone via the adrenal pathway and dihydrotestosterone (DHT) via the backdoor pathway, a 5α-reductase (SRD5A) inhibitor to diminish testosterone reduction to DHT and backdoor metabolism of progesterone substrates to DHT, and a newer antiandrogen to compete better with DHT for the androgen receptor ligand-binding domain. Early initiation of androgen annihilation for induction as part of planned intermittent ADT should be safe, may reduce tumor burden below a threshold that allows eradication by the immune system, and may cure many men who have failed definitive local therapy. © 2014 American Cancer Society.

  17. Development of a pico-second life-time spectrometer for positron annihilation studies

    International Nuclear Information System (INIS)

    Pujari, P.K.; Datta, T.; Tomar, B.S.; Das, S.K.

    1992-01-01

    Positron annihilation technique is a sensitive probe to investigate various physico-chemical phenomena due to the ability to provide information about the electron momentum and density in any medium. While measurements on the Doppler broadening and angular correlation of annihilation photons provide information about the electron momentum, the electron density at the annihilation site is obtained, by the positron life-time measurement. This report describes the development, optimization and calibration of a high resolution life-time spectrometer (FWHM=230 ps), based on fast-fast coincidence technique, a relatively new concept in nuclear timing spectroscopy. (author). 4 refs., 9 figs., 1 tab

  18. Dark matter annihilation into right-handed neutrinos and the galactic center gamma-ray excess

    Energy Technology Data Exchange (ETDEWEB)

    Tang, Yi-Lei [Center for High Energy Physics, Peking University,Beijing 100871 (China); Zhu, Shou-hua [Center for High Energy Physics, Peking University,Beijing 100871 (China); Institute of Theoretical Physics State Key Laboratory of Nuclear Physics and Technology,Peking University, Beijing 100871 (China); Collaborative Innovation Center of Quantum Matter,Beijing 100871 (China)

    2016-03-08

    In this paper, we will discuss a specific case that the dark matter particles annihilate into right-handed neutrinos. We calculate the predicted gamma-ray excess from the galactic center and compare our results with the data from the Fermi-LAT. An approximately 10–60 GeV right-handed neutrino with heavier dark matter particle can perfectly explain the observed spectrum. The annihilation cross section 〈σv〉 falls within the range 0.5–4×10{sup −26} cm{sup 3}/s, which is roughly compatible with the WIMP annihilation cross section.

  19. Coherent creation and annihilation of rotational wave packets in incoherent ensembles

    International Nuclear Information System (INIS)

    Lee, Kevin F.; Corkum, P. B.; Shapiro, E. A.; Villeneuve, D. M.

    2006-01-01

    Laser pulses can create rotational wave packets in molecules that periodically revive as field-free aligned distributions. These rotational wave packets can be approximately annihilated by applying another laser pulse during a half revival, an effect corresponding to quantum antiresonance in chaotic kicked rotor studies. We theoretically explore causes of deviation from perfect annihilation. We experimentally demonstrate rotational wave packet annihilation in nitrogen gas, measuring the evolution of alignment by Coulomb explosion imaging. As a test, we apply the pulse pair to an existing rotational wave packet and observe the restoration of the original revival structure after the zero-effect pulse pair

  20. Studying the recovery of as-received industrial Al alloys by positron annihilation spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Abdel-Hady, E.E. [Physics Department, Faculty of Science, El-Minia University, BO 61519, El-Minia (Egypt)]. E-mail: esamhady@link.net; Ashry, A. [Faculty of Education, Ain Shams University, Cairo (Egypt); Ismail, H. [Faculty of Education, Ain Shams University, Cairo (Egypt); El-Gamal, S. [Faculty of Education, Ain Shams University, Cairo (Egypt)

    2006-02-28

    Positron annihilation lifetime (PAL) spectroscopy, Doppler broadening of annihilation radiation (DBAR) spectroscopy and Vickers microhardness (Hv) measurements were performed to study the micro- and macro-structure variations during isochronal annealing from room temperature (RT) to 500 deg. Cof commercial pure Al (1 1 0 0), Al-Mn-Mg (3 0 0 4) and Al-Mg-Si (6 2 0 1) alloys. Three annealing stages of microstructures have been identified as recovery, partial recrystallization and complete recrystallization followed by grain growth. A positive correlation between the macroscopic mechanical properties (Hv) and positron annihilation parameters has been achieved for the three samples under investigation.

  1. Direct Detection Phenomenology in Models Where the Products of Dark Matter Annihilation Interact with Nuclei

    DEFF Research Database (Denmark)

    Cherry, John F.; Frandsen, Mads T.; Shoemaker, Ian M.

    2015-01-01

    We investigate the direct detection phenomenology of a class of dark matter (DM) models in which DM does not directly interact with nuclei, {but rather} the products of its annihilation do. When these annihilation products are very light compared to the DM mass, the scattering in direct detection...... to nuclei, the limit from annihilation to relativistic particles in the Sun can be stronger than that of conventional non-relativistic direct detection by more than three orders of magnitude for masses in a 2-7 GeV window....

  2. Revisiting big-bang nucleosynthesis constraints on dark-matter annihilation

    Directory of Open Access Journals (Sweden)

    Masahiro Kawasaki

    2015-12-01

    Full Text Available We study the effects of dark-matter annihilation during the epoch of big-bang nucleosynthesis on the primordial abundances of light elements. We improve the calculation of the light-element abundances by taking into account the effects of anti-nucleons emitted by the annihilation of dark matter and the interconversion reactions of neutron and proton at inelastic scatterings of energetic nucleons. Comparing the theoretical prediction of the primordial light-element abundances with the latest observational constraints, we derive upper bounds on the dark-matter pair-annihilation cross section. Implication to some of particle-physics models are also discussed.

  3. INTEGRAL SPI Limits on Electron-Positron Annihilation Radiation from the Galactic Plane

    DEFF Research Database (Denmark)

    Teegarden, B. J.; Watanabe, K.; Jean, P.

    2005-01-01

    The center of our Galaxy is a known strong source of electron‐positron 511 keV annihilation radiation. Thus far, however, there have been no reliable detections of annihilation radiation outside of the central radian of our Galaxy. One of the primary objectives of the INTEGRAL (International Gamma...... the first 10 months of observation. During this period a significant fraction of the observing time was spent in or near the Galactic plane. No positive annihilation flux was detected outside of the central region () of our Galaxy. In this paper we describe the observations and data analysis methods...

  4. Observation of rapid exciton-exciton annihilation in monolayer molybdenum disulfide.

    Science.gov (United States)

    Sun, Dezheng; Rao, Yi; Reider, Georg A; Chen, Gugang; You, Yumeng; Brézin, Louis; Harutyunyan, Avetik R; Heinz, Tony F

    2014-10-08

    Monolayer MoS2 is a direct-gap two-dimensional semiconductor that exhibits strong electron-hole interactions, leading to the formation of stable excitons and trions. Here we report the existence of efficient exciton-exciton annihilation, a four-body interaction, in this material. Exciton-exciton annihilation was identified experimentally in ultrafast transient absorption measurements through the emergence of a decay channel varying quadratically with exciton density. The rate of exciton-exciton annihilation was determined to be (4.3 ± 1.1) × 10(-2) cm(2)/s at room temperature.

  5. The influence of the "cage" effect on the mechanism of reversible bimolecular multistage chemical reactions proceeding from different sites in solutions.

    Science.gov (United States)

    Doktorov, Alexander B

    2016-08-28

    Manifestations of the "cage" effect at the encounters of reactants have been theoretically treated on the example of multistage reactions (including bimolecular exchange reactions as elementary stages) proceeding from different active sites in liquid solutions. It is shown that for reactions occurring near the contact of reactants, consistent consideration of quasi-stationary kinetics of such multistage reactions (possible in the framework of the encounter theory only) can be made on the basis of chemical concepts of the "cage complex," just as in the case of one-site model described in the literature. Exactly as in the one-site model, the presence of the "cage" effect gives rise to new channels of reactant transformation that cannot result from elementary event of chemical conversion for the given reaction mechanism. Besides, the multisite model demonstrates new (as compared to one-site model) features of multistage reaction course.

  6. Annihilation vs. Decay: Constraining dark matter properties from a gamma-ray detection

    CERN Document Server

    Palomares-Ruiz, Sergio

    2010-01-01

    Most proposed dark matter candidates are stable and are produced thermally in the early Universe. However, there is also the possibility of unstable (but long-lived) dark matter, produced thermally or otherwise. We propose a strategy to distinguish between dark matter annihilation and/or decay in the case that a clear signal is detected in gamma-ray observations of Milky Way dwarf spheroidal galaxies with current or future gamma-ray experiments. The sole measurement of the energy spectrum of an indirect signal would render the discrimination between these cases impossible. We show that by examining the dependence of the intensity and energy spectrum on the angular distribution of the emission, the origin could be identified as decay, annihilation, or both. In addition, once the type of signal is established, we show how these measurements could help to extract information about the dark matter properties, including mass, annihilation cross section, lifetime, dominant annihilation and decay channels, and the p...

  7. Probing dark matter annihilation in the Galaxy with antiprotons and gamma rays

    Energy Technology Data Exchange (ETDEWEB)

    Cuoco, Alessandro; Heisig, Jan; Korsmeier, Michael; Krämer, Michael, E-mail: cuoco@physik.rwth-aachen.de, E-mail: heisig@physik.rwth-aachen.de, E-mail: korsmeier@physik.rwth-aachen.de, E-mail: mkraemer@physik.rwth-aachen.de [Institute for Theoretical Particle Physics and Cosmology, RWTH Aachen University, 52056 Aachen (Germany)

    2017-10-01

    A possible hint of dark matter annihilation has been found in Cuoco, Korsmeier and Krämer (2017) from an analysis of recent cosmic-ray antiproton data from AMS-02 and taking into account cosmic-ray propagation uncertainties by fitting at the same time dark matter and propagation parameters. Here, we extend this analysis to a wider class of annihilation channels. We find consistent hints of a dark matter signal with an annihilation cross-section close to the thermal value and with masses in range between 40 and 130 GeV depending on the annihilation channel. Furthermore, we investigate in how far the possible signal is compatible with the Galactic center gamma-ray excess and recent observation of dwarf satellite galaxies by performing a joint global fit including uncertainties in the dark matter density profile. As an example, we interpret our results in the framework of the Higgs portal model.

  8. Magnetic Field Effects on Triplet-Triplet Annihilation in Solutions: Modulation of Visible/NIR Luminescence

    Science.gov (United States)

    Mani, Tomoyasu; Vinogradov, Sergei A.

    2013-01-01

    Photon upconversion based on sensitized triplet-triplet annihilation (TTA) presents interest for such areas as photovoltaics and imaging. Usually energy upconversion is observed as p-type delayed fluorescence from molecules whose triplet states are populated via energy transfer from a suitable triplet donor, followed by TTA. Magnetic field effects (MFE) on delayed fluorescence in molecular crystals are well known; however, there exist only a few examples of MFE on TTA in solutions, and all of them are limited to UV-emitting materials. Here we present MFE on TTA-mediated visible and near infrared (NIR) emission, sensitized by far-red absorbing metalloporphyrins in solutions at room temperature. In addition to visible delayed fluorescence from annihilator, we also observed NIR emission from the sensitizer, occurring as a result of triplet-triplet energy transfer back from annihilator, termed “delayed phosphorescence”. This emission also exhibits MFE, but opposite in sign to the annihilator fluorescence. PMID:24143268

  9. Kinetics of Schottky defect formation and annihilation in single crystal TlBr.

    Science.gov (United States)

    Bishop, Sean R; Tuller, Harry L; Kuhn, Melanie; Ciampi, Guido; Higgins, William; Shah, Kanai S

    2013-07-28

    The kinetics for Schottky defect (Tl and Br vacancy pair) formation and annihilation in ionically conducting TlBr are characterized through a temperature induced conductivity relaxation technique. Near room temperature, defect generation-annihilation was found to take on the order of hours before equilibrium was reached after a step change in temperature, and that mechanical damage imparted on the sample rapidly increases this rate. The rate limiting step to Schottky defect formation-annihilation is identified as being the migration of lower mobility Tl (versus Br), with an estimate for source-sink density derived from calculated diffusion lengths. This study represents one of the first investigations of Schottky defect generation-annihilation kinetics and demonstrates its utility in quantifying detrimental mechanical damage in radiation detector materials.

  10. Positron annihilation characteristics in multi-wall carbon nanotubes with different average diameters

    International Nuclear Information System (INIS)

    Tuyen, L A; Khiem, D D; Phuc, P T; Kajcsos, Zs; Lázár, K; Tap, T D

    2013-01-01

    Positron lifetime spectroscopy was used to study multi-wall carbon nanotubes. The measurements were performed in vacuum on the samples having different average diameters. The positron lifetime values depend on the nanotube diameter. The results also show an influence of the nanotube diameter on the positron annihilation intensity on the nanotube surface. The change in the annihilation probability is described and interpreted by the modified diffusion model introducing the positron escape rate from the nanotubes to their external surface.

  11. Annihilation diagrams in two-body nonleptonic decays of charmed mesons

    International Nuclear Information System (INIS)

    Bedaque, P.; Das, A.; Mathur, V.S.

    1994-06-01

    In the pole-dominance model for the two-body nonleptonic decays of charmed mesons D → PV and D → VV, it is shown that the contributions of the intermediate pseudoscalar and the axial-vector meson poles cancel each other in the annihilation diagrams in the chiral limit. In the same limit, the annihilation diagrams for the D → PP decays vanish independently. (author). 6 refs, 3 figs

  12. Bubble detector measurements of a mixed radiation field from antiproton annihilation

    DEFF Research Database (Denmark)

    Bassler, Niels; Knudsen, Helge; Møller, Søren Pape

    2006-01-01

    In the light of recent progress in the study of the biological potential of antiproton tumour treatment it is important to be able to characterize the neutron intensity arising from antiproton annihilation using simple, compact and reliable detectors. The intensity of fast neutrons from antiproton...... annihilation on polystyrene has been measured with bubble detectors and a multiplicity has been derived as well as an estimated neutron equivalent dose. Additionally the sensitivity of bubble detectors towards protons was measured....

  13. Measurement of the antiproton-nucleus annihilation cross-section at low energy

    Science.gov (United States)

    Aghai-Khozani, H.; Bianconi, A.; Corradini, M.; Hayano, R.; Hori, M.; Leali, M.; Lodi Rizzini, E.; Mascagna, V.; Murakami, Y.; Prest, M.; Vallazza, E.; Venturelli, L.; Yamada, H.

    2018-02-01

    Systematic measurements of the annihilation cross sections of low energy antinucleons were performed at CERN in the 80's and 90's. However the antiproton data on medium-heavy and heavy nuclear targets are scarce. The ASACUSA Collaboration at CERN has measured the antiproton annihilation cross section on carbon at 5.3 MeV: the value is (1.73 ± 0.25) barn. The result is compared with the antineutron experimental data and with the theoretical previsions.

  14. Differences between annihilation and nonannihilation characteristics of anti pp-interactions at 22.4 GeV/c

    International Nuclear Information System (INIS)

    Batyunya, B.V.; Boguslavsky, I.V.; Gramenitsky, I.M.; Lednicky, R.; Vrba, V.; Zlatanov, Z.; Fillipova, V.V.; Samoilov, V.V.; Temiraliev, T.; Levonian, S.V.; Villanen, P.; Walck, E.; Dementiev, R.K.; Korzhavina, I.A.; Leikin, E.M.; Puzyrnyi, A.G.; Rud, V.I.; Tikhonova, L.A.; Herynek, I.; Lokajicek, M.; Ridky, J.; Simak, V.; Leitner, R.; Suk, M.; Valkarova, A.; Kuratashvili, G.O.; Topuria, T.P.; Tsintsadze, V.D.

    1985-01-01

    All anti pp events at 22.4 GeV/c were separated into nonannihilation (N-group) and enriched annihilation (A-group) events. The mean sphericity value for the A-sample is in accordance with e + e - , K - p and π - p data. The experimental value of for events from the A-sample is larger than the value for N-events for all multiplicities. Mean charge transfer is found to be very sensitive to the dynamics of the process. The experimental value of mean charge transfer is = -0.25 if possible particle misidentification is taken into account. The experimental data are compared with the quark-parton model predictions. (orig.)

  15. Proton-antiproton annihilation into a lambdaC-antiLambdaC pair within the generalized parton picture

    International Nuclear Information System (INIS)

    Goritschnig, A. T.

    2009-01-01

    The proton-antiproton annihilation into a LambdaC-AntiLambdaC pair is investigated within the handbag approach. It is shown that the dominant dynamical mechanism, characterized by the partonic subprocess anti-u u -> anti-c c, factorizes in the sense that only the subprocess contains highly virtual partons, a gluon to lowest order of perturbative QCD, while the hadronic matrix elements embody only soft scales and can be parameterized in terms of helicity flip and non-flip generalized parton distributions. Modelling these parton distributions by overlaps of light-cone wave functions for the involved baryons were able to predict cross sections and spin correlation parameters for the process of interest. (author) [de

  16. Mode coupling and multiquantum vibrational excitations in Feshbach-resonant positron annihilation in molecules

    Science.gov (United States)

    Gribakin, G. F.; Stanton, J. F.; Danielson, J. R.; Natisin, M. R.; Surko, C. M.

    2017-12-01

    The dominant mechanism of low-energy positron annihilation in polyatomic molecules is through positron capture in vibrational Feshbach resonances (VFR). In this paper, we investigate theoretically the effect of anharmonic terms in the vibrational Hamiltonian on positron annihilation rates. Such interactions enable positron capture in VFRs associated with multiquantum vibrational excitations, leading to enhanced annihilation. Mode coupling can also lead to faster depopulation of VFRs, thereby reducing their contribution to the annihilation rates. To analyze this complex picture, we use coupled-cluster methods to calculate the anharmonic vibrational spectra and dipole transition amplitudes for chloroform, chloroform-d1, 1,1-dichloroethylene, and methanol, and use these data to compute positron resonant annihilation rates for these molecules. Theoretical predictions are compared with the annihilation rates measured as a function of incident positron energy. The results demonstrate the importance of mode coupling in both enhancement and suppression of the VFR. There is also experimental evidence for the direct excitation of multimode VFR. Their contribution is analyzed using a statistical approach, with an outlook towards more accurate treatment of this phenomenon.

  17. Hunting for glueballs in electron-positron annihilation.

    Science.gov (United States)

    Brodsky, Stanley J; Goldhaber, Alfred Scharff; Lee, Jungil

    2003-09-12

    We calculate the cross section for the exclusive production of J(PC)=0(++) glueballs G0 in association with the J/psi in e(+)e(-) annihilation using the perturbative QCD factorization formalism. The required long-distance matrix element for the glueball is bounded by CUSB data from a search for resonances in radiative Upsilon decay. The cross section for e(+)e(-)-->J/psi+G0 at sqrt[s]=10.6 GeV is similar to exclusive charmonium-pair production e(+)e(-)-->J/psi+h for h=eta(c) and chi(c0), and is larger by a factor of 2 than that for h=eta(c)(2S). As the subprocesses gamma(*)-->(cc)(cc) and gamma(*)-->(cc)(gg) are of the same nominal order in perturbative QCD, it is possible that some portion of the anomalously large signal observed by Belle in e(+)e(-)-->J/psiX may actually be due to the production of charmonium-glueball J/psiG(J) pairs.

  18. Positron Annihilation Study of Ion-irradiated Si

    International Nuclear Information System (INIS)

    Shin, Jung Ki; Kwon, Jun Hyun; Lee, Jong Yong

    2009-01-01

    Structural parts like a spaceship, satellite and solar cell are composed of metal alloy or semiconductor materials. Especially, Si is used as a primary candidate alloy. But, manned and robotic missions to the Earth's moon and Mars are exposed to a continuous flux of Galactic Cosmic Rays (GCR) and occasional, but intense, fluxes of Solar Energetic Particles. These natural radiations impose hazards to manned exploration. Irradiation of cosmic particle induces various changes in the mechanical and physical properties of device steels. It is, therefore, important to investigate radiation damage to the component materials in semiconductor. The evolution of radiation-induced defects leads to degradation of the mechanical properties. One of them includes irradiation embrittlement, which can cause a loss of ductility and further increase the probability of a brittle fracture. It can be more dangerous in the space. Positron annihilation lifetime spectroscopy(PALS) have been applied to investigate the production of vacancy-type defects for Ion-irradiated Si wafer penetrated by H, He, O and Fe ions. Then, we carried out a comparison with an un-irradiated Si wafer

  19. Positron annihilation lifetime spectroscopy of ZnO bulk samples

    International Nuclear Information System (INIS)

    Zubiaga, A.; Plazaola, F.; Garcia, J. A.; Tuomisto, F.; Munoz-Sanjose, V.; Tena-Zaera, R.

    2007-01-01

    In order to gain a further insight into the knowledge of point defects of ZnO, positron annihilation lifetime spectroscopy was performed on bulk samples annealed under different atmospheres. The samples were characterized at temperatures ranging from 10 to 500 K. Due to difficulties in the conventional fitting of the lifetime spectra caused by the low intensity of the defect signals, we have used an alternative method as a solution to overcome these difficulties and resolve all the lifetime components present in the spectra. Two different vacancy-type defects are identified in the samples: Zn vacancy complexes (V Zn -X) and vacancy clusters consisting of up to five missing Zn-O pairs. In addition to the vacancies, we observe negative-ion-type defects, which are tentatively attributed to intrinsic defects in the Zn sublattice. The effect of the annealing on the observed defects is discussed. The concentrations of the V Zn -X complexes and negative-ion-type defects are in the 0.2-2 ppm range, while the cluster concentrations are 1-2 orders of magnitude lower

  20. The role of positronium decoherence in positron annihilation in matter

    Energy Technology Data Exchange (ETDEWEB)

    Pietrow, M., E-mail: mrk@kft.umcs.lublin.pl [Institute of Physics, M. Curie-Sklodowska University, ul. Pl. M. Curie-Sklodowskiej 1, 20-031 Lublin (Poland); Slomski, P. [Geographic Information Systems Development Company Martinex, ul. Melgiewska 95, 21-040 Swidnik (Poland)

    2011-10-24

    A small difference between the energies of the para-positronium (p-Ps) and ortho-positronium (o-Ps) states suggests the possibility of the superposition of p-Ps and o-Ps during the formation of positronium (Ps) from pre-Ps, terminating its migration in the matter in a void. It is shown that such a superposition decoheres in the basis of p-Ps and o-Ps. The decoherence time scale estimated here motivates a correction in the precise analysis of the positron annihilation lifetime spectra. More generally, the superposited Ps state should contribute to the theory of the evolution of positronium in matter. -- Highlights: → Decoherence time decrease exponentially with the number of e{sup -} interacting with Ps. → Time scale of the decoherence motivates correction in decomposition of PALS spectra. → We showed the way of modification for formulas used for PALS spectra decomposition. → The superposited Ps should contribute to the positronium in matter evolution theory. → We examined the magnetisation influence to be expected on the process of decoherence.

  1. Pore Topology Effects in Positron Annihilation Spectroscopy of Zeolites.

    Science.gov (United States)

    Zubiaga, Asier; Warringham, Robbie; Mitchell, Sharon; Gerchow, Lars; Cooke, David; Crivelli, Paolo; Pérez-Ramírez, Javier

    2017-03-03

    Positron annihilation spectroscopy (PAS) is a powerful method to study the size and connectivity of pores in zeolites. The lifetime of positronium within the host material is commonly described by the Tao-Eldrup model. However, one of its largest limitations arises from the simple geometries considered for the shape of the pores, which cannot describe accurately the complex topologies in zeolites. Here, an atomic model that combines the Tao potential with the crystallographic structure is introduced to calculate the distribution and lifetime of Ps intrinsic to a given framework. A parametrization of the model is undertaken for a set of widely applied zeolite framework types (*BEA, FAU, FER, MFI, MOR, UTL), before extending the model to all known structures. The results are compared to structural and topological descriptors, and to the Tao-Eldrup model adapted for zeolites, demonstrating the intricate dependence of the lifetime on the pore architecture. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

  2. Molecular pathways for defect annihilation in directed self-assembly

    Science.gov (United States)

    Hur, Su-Mi; Thapar, Vikram; Ramírez-Hernández, Abelardo; Khaira, Gurdaman; Segal-Peretz, Tamar; Rincon-Delgadillo, Paulina A.; Li, Weihua; Müller, Marcus; Nealey, Paul F.; de Pablo, Juan J.

    2015-01-01

    Over the last few years, the directed self-assembly of block copolymers by surface patterns has transitioned from academic curiosity to viable contender for commercial fabrication of next-generation nanocircuits by lithography. Recently, it has become apparent that kinetics, and not only thermodynamics, plays a key role for the ability of a polymeric material to self-assemble into a perfect, defect-free ordered state. Perfection, in this context, implies not more than one defect, with characteristic dimensions on the order of 5 nm, over a sample area as large as 100 cm2. In this work, we identify the key pathways and the corresponding free energy barriers for eliminating defects, and we demonstrate that an extraordinarily large thermodynamic driving force is not necessarily sufficient for their removal. By adopting a concerted computational and experimental approach, we explain the molecular origins of these barriers and how they depend on material characteristics, and we propose strategies designed to overcome them. The validity of our conclusions for industrially relevant patterning processes is established by relying on instruments and assembly lines that are only available at state-of-the-art fabrication facilities, and, through this confluence of fundamental and applied research, we are able to discern the evolution of morphology at the smallest relevant length scales—a handful of nanometers—and present a view of defect annihilation in directed self-assembly at an unprecedented level of detail. PMID:26515095

  3. Tests der pertubativen QCD in der e+e Annihilation

    CERN Document Server

    Passon, Oliver

    2002-01-01

    This thesis presents the DELPHI measurement of event shape distributions and inclusive spectra in e+e- annihilation at LEP between 183 and 207 GeV. These data have been reprocessed in 2001 and the results supersede some older DELPHI measurements at the corresponding energies [1, 2, 3, 4, 5]. The differential distributions in Ep = ln 1/xp and their maxima E* are compared with predictions in the MLLA/LPHD framework. These tests support the manifestation of coherence effects on the hadronic level. From the event shapes Thrust, C parameter heavy jet mass wide and total jet broadening s is extracted with four different methods: The differential distributions are compared to predictions in O s pure NLLA and O s + NLLA logR folded with fragmentation models For the mean values s is extracted using an analytical power correction ansatz. The s values are combined with results obtained at other LEP energies and at and around MZ This allows both a combined measurement of s and a test of the running of s The smallest unce...

  4. Miracle on the Vistula: The Red Army’s Failure and the Birth of the Deep Operations Theory of Annihilation

    Science.gov (United States)

    2017-04-09

    Miracle on the Vistula: The Red Army’s Failure and the Birth of the Deep Operations Theory of Annihilation A Monograph by MAJ Charles E. Thompson...Vistula: The Red Army’s Failure and the Birth of the Deep Operations Theory of Annihilation 5a. CONTRACT NUMBER 5b. GRANT NUMBER 5c. PROGRAM...victory in World War II: the Deep Operations Theory of Annihilation . This monograph seeks to explore the impact of the war with Poland and its

  5. Pore annihilation in a single-crystal nickel-base superalloy during hot isostatic pressing: Experiment and modelling

    International Nuclear Information System (INIS)

    Epishin, Alexander; Fedelich, Bernard; Link, Thomas; Feldmann, Titus; Svetlov, Igor L.

    2013-01-01

    Pore annihilation during hot isostatic pressing (HIP) was investigated in the single-crystal nickel-base superalloy CMSX-4 experimentally by interrupted HIP tests at 1288 °C/103 MPa. The kinetics of pore annihilation was determined by density measurement and quantitative metallography. Transmission electron microscopy of a HIPed specimen showed that the pores shrink via dislocation movement on octahedral glide planes. Theoretically pore closure under HIP condition was modelled by the finite element method using crystal plasticity and large strain theories. The modelling gives a similar kinetics of pore annihilation as observed experimentally, however somewhat higher annihilation rate

  6. Positron annihilation studies on chalcone chromophore doped PVA

    Energy Technology Data Exchange (ETDEWEB)

    Bhajantri, R.F.; Ravindrachary, V.; Harisha, A.; Ismayil [Department of Physics, Mangalore University, Mangalagangotri (India); Ranganathaiah, C. [Department of Studies in Physics, University of Mysore, Manasagangotri (India)

    2009-11-15

    A novel organic non-linear optical material 1-(4-methylphenyl)-3-(4- N, N dimethyl amino phenyl)-2-propen-1-one (MPDMAPP) chalcone chromophore has been synthesized by standard method. Pure and MPDMAPP doped Poly(vinyl alcohol) films are prepared using solution casting method and characterized using UV-Visible absorption and Positron Annihilation Lifetime Spectroscopy. The optical spectroscopic study shows three absorption bands, 196-202 nm assigned to localized n {yields}{pi}* transitions, 205-320 nm to n {yields}{pi} inter-band and 385-428 nm assigned to {pi} {yields}{pi}* transition and arises due to the charge transfer complex. Using observed UV-Vis spectra, three optical energy gaps, E{sub g1} (4.96-4.25 eV), E{sub g2} (3.47-3.32 eV) and E{sub g3} (2.33-2.24 eV) have been estimated. The observed change in E{sub g} upon doping is understood based on the formation of charge transfer complex arising from the -HC=CH- structure present in the composite and due to the interactions of dopant and OH group of PVA. The PALS results shows that the o-Ps lifetime decreases continuously as doping concentration increases and I{sub 3} initially increases (from 18.82% to 20.95%) from 0 wt% to 0.05 wt% and then decreases gradually up to 16.76% for higher dopant concentrations with decrease in optical band gaps. The variation of positron data with E{sub g} is understood by correlating the probability of Ps formation with the complex. (copyright 2009 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

  7. Positron annihilation lifetime study of radiation-damaged natural zircons

    Energy Technology Data Exchange (ETDEWEB)

    Roberts, J. [Centre for Antimatter-Matter Studies, Research School of Physics and Engineering, The Australian National University, Canberra (Australia); Gaugliardo, P. [Centre for Antimatter-Matter Studies, School of Physics, University of Western Australia (Australia); Farnan, I.; Zhang, M. [Department of Earth Sciences, University of Cambridge (United Kingdom); Vance, E.R.; Davis, J.; Karatchevtseva, I.; Knott, R.B. [Australian Nuclear Science and Technology Organisation (Australia); Mudie, S. [The Australian Synchrotron, Victoria (Australia); Buckman, S.J. [Centre for Antimatter-Matter Studies, Research School of Physics and Engineering, The Australian National University, Canberra (Australia); Institute for Mathematical Sciences, University of Malaya, Kuala Lumpur (Malaysia); Sullivan, J.P., E-mail: james.sullivan@anu.edu.au [Centre for Antimatter-Matter Studies, Research School of Physics and Engineering, The Australian National University, Canberra (Australia)

    2016-04-01

    Zircons are a well-known candidate waste form for actinides and their radiation damage behaviour has been widely studied by a range of techniques. In this study, well-characterised natural single crystal zircons have been studied using Positron Annihilation Lifetime Spectroscopy (PALS). In some, but not all, of the crystals that had incurred at least half of the alpha-event damage of ∼10{sup 19} α/g required to render them structurally amorphous, PALS spectra displayed long lifetimes corresponding to voids of ∼0.5 nm in diameter. The long lifetimes corresponded to expectations from published Small-Angle X-ray Scattering data on similar samples. However, the non-observation by PALS of such voids in some of the heavily damaged samples may reflect large size variations among the voids such that no singular size can be distinguished or. Characterisation of a range of samples was also performed using scanning electron microscopy, optical absorption spectroscopy, Raman scattering and X-ray scattering/diffraction, with the degree of alpha damage being inferred mainly from the Raman technique and X-ray diffraction. The observed void diameters and intensities of the long lifetime components were changed somewhat by annealing at 700 °C; annealing at 1200 °C removed the voids entirely. The voids themselves may derive from He gas bubbles or voids created by the inclusion of small quantities of organic and hydrous matter, notwithstanding the observation that no voidage was evidenced by PALS in two samples containing hydrous and organic matter. - Highlights: • Study of a range of naturally occurring zircons damaged by alpha radiation. • Characterised using a range of techniques, including PALS spectroscopy. • Effects on hydrous material appear important, rather than direct radiation damage. • Annealing is shown to remove the observed voids.

  8. Evaluation of the reactor pressure vessel steels by positron annihilation

    Energy Technology Data Exchange (ETDEWEB)

    Slugeň, V., E-mail: Vladimir.Slugen@elf.stuba.sk [Institute of Nuclear and Physical Engineering, Slovak University of Technology, Ilkovičova 3, 81219 Bratislava (Slovakia); Hein, H. [AREVA NP GmbH, Paul Gossen Strasse 100, 91 001 Erlangen (Germany); Sojak, S.; Simeg Veterníková, J.; Petriska, M.; Sabelová, V.; Pavúk, M.; Hinca, R.; Stacho, M. [Institute of Nuclear and Physical Engineering, Slovak University of Technology, Ilkovičova 3, 81219 Bratislava (Slovakia)

    2013-11-15

    This paper presents a comparison of commercially used German and Russian reactor pressure vessel steels from the positron annihilation spectroscopy (PAS) point of view, having in mind knowledge obtained also from other techniques from the last decades. The second generation of Russian RPV steels seems to be fully comparable with German steels and their quality allows prolongation of NPP operating lifetime over projected 40 years. The embrittlement of CrMoV steels is relatively low due to effect of higher temperature which implies partial in situ annealing of primary microstructural point defects and therefore delays the degradation processes caused by neutron irradiation. PAS techniques can be effectively applied for evaluation of microstructural changes caused by extreme external loads (characterized by high dpa values) by proton implantation, with aim to simulate irradiation and for the evaluation of the effectiveness of post-irradiation thermal treatments. We used our actual and previous results, collected during last 20 years from measurements of different RPV-steels in “as received”, irradiated and post-irradiation annealed state and compare them with the aim to contribute to general knowledge based on experimental PAS data. Actual results from irradiated German and Russian steels confirmed that no large voids or vacancy clusters were formed at defined irradiation conditions stated according to the real operational conditions at nuclear power plants. This indicate the fact that vacancy type defects bear hardly any responsibility for radiation-induced hardening and embrittlement of reactor pressure vessel steels and does not affect significantly the long-term operation of nuclear power plants from safety point of view.

  9. A systematic effective operator analysis of semi-annihilating dark matter

    Energy Technology Data Exchange (ETDEWEB)

    Cai, Yi [ARC Centre of Excellence for Particle Physics at the Terascale, School of Physics,The University of Melbourne,Melbourne, Victoria 3010 (Australia); Spray, Andrew [Center for Theoretical Physics of the Universe, Institute for Basic Science (IBS),Daejeon, 34051 (Korea, Republic of)

    2017-02-23

    Semi-annihilation is a generic feature of dark matter theories stabilized by symmetries larger than a ℤ{sub 2}. It contributes to thermal freeze out, but is irrelevant for direct and collider searches. This allows semi-annihilating dark matter to avoid those limits in a natural way. We use an effective operator approach to make the first model-independent study of the associated phenomenology. We enumerate all possible operators that contribute to 2→2 semi-annihilation up to dimension 6, plus leading terms at dimension 7. We find that when the only light states charged under the dark symmetry are dark matter, the model space is highly constrained. Only fifteen operators exist, and just two for single-component dark sectors. If there can be additional light, unstable “dark partner” states the possible phenomenology greatly increases, at the cost of additional model dependence in the dark partner decay modes. We also derive the irreducible constraints on models with single-component dark matter from cosmic ray searches and astrophysical observations. We find that for semi-annihilation to electrons and light quarks, the thermal relic cross sections can be excluded for dark matter masses up to 100 GeV. However, significant model space for semi-annihilating dark matter remains.

  10. Positron Annihilation in Carbon Nanotubes Studied by Coincidence Doppler Broadening Spectroscopy

    Science.gov (United States)

    Murakami, H.; Sato, K.; Kanazawa, I.; Sano, M.

    2008-05-01

    In order to assign the sites of positron annihilation, coincidence Doppler broadening spectra were measured for a highly oriented pyrolytic graphite crystal, graphite powder, multi-walled carbon nanotubes (MNTs) and cup-stacked carbon nanotubes (CNTs). The spectrum for graphite powder normalized to that for highly oriented pyrolytic graphite (HOPG) is almost flat in the momentum region from 7×10-3 to 13×10-3 mec, having a ratio close to unity. The flat spectrum demonstrates that positrons injected into graphite powder annihilate in the interlayer spaces of piled graphite sheets, in the same manner as positrons in highly oriented pyrolytic graphite annihilate in the bulk. The coincidence Doppler broadening spectra for MNTs and CNTs are quite different from that for highly oriented pyrolytic graphite, which indicates that positrons injected into MNTs and CYTs annihilate not in the bulk, but on surface. The positron lifetime spectrum for multi-walled carbon nanotubes is analyzed in terms of a single component due to surface-trapped positrons, while that for CNTs is decomposed into three components attributable to para-positronium surface-trapped positrons and ortho-positronium. The difference between the coincidence Doppler broadening spectrum for CNTs and that for MNTs is explained in terms of positron annihilation on zigzag surfaces of CNTs which are composed of both graphite-sheet and graphite-edge planes.

  11. A systematic effective operator analysis of semi-annihilating dark matter

    International Nuclear Information System (INIS)

    Cai, Yi; Spray, Andrew

    2017-01-01

    Semi-annihilation is a generic feature of dark matter theories stabilized by symmetries larger than a ℤ 2 . It contributes to thermal freeze out, but is irrelevant for direct and collider searches. This allows semi-annihilating dark matter to avoid those limits in a natural way. We use an effective operator approach to make the first model-independent study of the associated phenomenology. We enumerate all possible operators that contribute to 2→2 semi-annihilation up to dimension 6, plus leading terms at dimension 7. We find that when the only light states charged under the dark symmetry are dark matter, the model space is highly constrained. Only fifteen operators exist, and just two for single-component dark sectors. If there can be additional light, unstable “dark partner” states the possible phenomenology greatly increases, at the cost of additional model dependence in the dark partner decay modes. We also derive the irreducible constraints on models with single-component dark matter from cosmic ray searches and astrophysical observations. We find that for semi-annihilation to electrons and light quarks, the thermal relic cross sections can be excluded for dark matter masses up to 100 GeV. However, significant model space for semi-annihilating dark matter remains.

  12. Assessment of positron annihilation as a potential non-destructive examination technique

    International Nuclear Information System (INIS)

    Jones, W.B.; Van Den Avyle, J.A.; Gauster, W.B.; Wampler, W.R.

    1979-01-01

    The positron annihilation technique can provide a sensitive measure of defect density in metals. In this program the technique has been used to monitor defects generated during plastic deformation by cold work or fatigue cycling. The primary goals have been: (1) to assess the degree of sensitivity of the technique; (2) to correlate positron annihilation readings with observed microstructural changes to better understand the physical basis for these readings; and (3) to determine correlations between positron annihilation measurements and number of fatigue cycles. Examination of fatigued samples by transmission electron microscopy indicates some correlation between dislocation density and positron annihilation lineshape parameter (determined by the Doppler broadening technique). However, annealing studies of deformed samples indicate that positron annihilation response in 316 stainless steel is sensitive primarily to excess vacancies generated during the deformation and is less sensitive to dislocation density. Data on deformed nickel show sensitivity to both vacancies and dislocations. In general, lineshape parameter values tend to achieve a constant level at approximately 10% of fatigue life

  13. Glass transition and relaxation processes of polymers studied by positron annihilation

    Energy Technology Data Exchange (ETDEWEB)

    Uedono, Akira; Tanigawa, Shoichiro [Tsukuba Univ., Ibaraki (Japan). Inst. of Materials Science

    1996-10-01

    The glass transition and relaxation processes of polymers were studied by the positron annihilation technique. A positron implanted into polymers might annihilate from positronium (Ps) states in open spaces. Ps is a bound state between a positron and an electron, and its nonrelativistic quantum mechanics is practically identical to that of a hydrogen atom. The lifetime of Ps can be associated with the size of the open spaces, and the formation probability of Ps provides information of motions of molecules. Since the glass transition or relaxation processes affect behavior of open spaces, one can study these phenomena through the detection of the open spaces using the positron annihilation technique. In the present paper, we report studies of the glass transition and relaxation processes in polyethylene, polypropylene, and polystyrene by measurements of lifetime spectra of positrons and those of Doppler broadening profiles of the annihilation radiation. For these specimens, by measurements of the lifetime of Ps, {tau}{sub 3}, as a function of temperature, the glass transition temperature, T{sub g}, was determined as an onset temperature of the increase in the temperature coefficient of {tau}{sub 3}. Below T{sub g}, local motions of molecules were detected by measurements of the formation probability of Ps. The positron annihilation as a tool for the characterization of polymers was discussed. (author). 51 refs.

  14. Compton backscattered annihilation line emission: A new diagnostic of accreting compact sources

    Science.gov (United States)

    Lingenfelter, Richard E.; Hua, Xin-Min

    1992-01-01

    It is shown that Compton scattering of 511 keV electron-positron annihilation radiation produces a line like feature at approx. 170 keV from backscattered photons. Assuming a simple model of an accretion disk around a compact source, the spectrum is explored of the spectrum of Compton scattered annihilation line emission for a range of conditions. It is further shown that such Compton baskscattering of annihilation line emission from the inner edge of an accretion disk could account for the previously unidentified 170 keV line emission and high energy continuum observed from a variable, compact source, or sources, of annihilation radiation near the Galactic Center. Identification of the observed 170 keV line as an annihilation line reflection feature provides strong new evidence that the source of the emission is an accreting compact object. Further study of these features in existing spectra and in forthcoming GRO observation of these and other sources can provide unique new diagnostics of the innermost regions of accretion disks around compact objects.

  15. Mn-Doping in NiO Nanoparticles: Defects-Modifications and Associated Effects Investigated Through Positron Annihilation Spectroscopy.

    Science.gov (United States)

    Das, Anjan; Mandal, Atis Chandra; Roy, Soma; Nambissan, P M G

    2016-04-01

    Manganese-doped nickel oxide (Ni1-xMnxO) nanoparticulate samples with x in the range 0 (undoped sample) to 0.35 were synthesized by sol-gel method involving chemical reactions between the solutions of nickel nitrate hexahydrate and manganese acetate tetrahydrate. The nanocrystallites obtained after annealing of the precipitates for different durations were characterized by X-ray diffraction and high resolution transmission electron microscopy. The samples showed high degree of purity with no secondary phase up to 35 at.% (x = 0.35) of Mn-doping. At the initial doping concentrations, the crystallite sizes increased due to vacancy type defects being recombined with some of the doped Mn2+ ions. However, substitution-induced strain soon overtook the crystallite dynamics and the sizes rapidly started reducing again as an indirect consequence of the necessity to accommodate majority of the doped cations on the surfaces of the nanocrystallites. There was conspicuous changes in the lattice parameter too which could again be attributed to the strain and charge effects. The average sizes of the crystallites were obtained in the range 5.5 nm to 13.1 nm for the different samples. UV-Vis absorption studies indicated the formation of excitonic states in NiO on Mn-doping. The band gap energy (Eg) derived from the optical absorption spectra showed a continuous increase with increase of Mn-doping of the samples. Positron lifetime and Doppler broadening spectroscopic studies were carried out on those samples to characterize the vacancy type defects and defect clusters/complexes. There were also indications to suggest positron annihilation at the crystallite surfaces owing to their sizes of nanometer order. Positron lifetimes decreased upon increase of Mn-doping. The coincidence Doppler broadened ratio curves indicated definite shifts of the prominent oxygen-electron-annihilation peak and the variation of the lineshape parameter S also indicated clearly the effects of Mn-doping.

  16. High energy resolution and first time-dependent positron annihilation induced Auger electron spectroscopty

    Energy Technology Data Exchange (ETDEWEB)

    Mayer, Jakob

    2010-04-03

    It was the aim of this thesis to improve the existing positron annihilation induced Auger spectrometer at the highly intense positron source NEPOMUC (NEutron induced POsitron source MUniCh) in several ways: Firstly, the measurement time for a single spectrum should be reduced from typically 12 h to roughly 1 h or even less. Secondly, the energy resolution, which amounted to {delta}E/E{approx}10%, should be increased by at least one order of magnitude in order to make high resolution positron annihilation induced Auger spectroscopy (PAES)-measurements of Auger transitions possible and thus deliver more information about the nature of the Auger process. In order to achieve these objectives, the PAES spectrometer was equipped with a new electron energy analyzer. For its ideal operation all other components of the Auger analysis chamber had to be adapted. Particularly the sample manipulation and the positron beam guidance had to be renewed. Simulations with SIMION {sup registered} ensured the optimal positron lens parameters. After the adjustment of the new analyzer and its components, first measurements illustrated the improved performance of the PAES setup: Firstly, the measurement time for short overview measurements was reduced from 3 h to 420 s. The measurement time for more detailed Auger spectra was shortened from 12 h to 80 min. Secondly, even with the reduced measurement time, the signal to noise ratio was also enhanced by one order of magnitude. Finally, the energy resolution was improved to {delta}E/E < 1. The exceptional surface sensitivity and elemental selectivity of PAES was demonstrated in measurements of Pd and Fe, both coated with Cu layers of varying thickness. PAES showed that with 0.96 monolayer of Cu on Fe, more than 55% of the detected Auger electrons stem from Cu. In the case of the Cu coated Pd sample 0.96 monolayer of Cu resulted in a Cu Auger fraction of more than 30% with PAES and less than 5% with electron induced Auger spectroscopy

  17. Live cell imaging of interactions between replicase and capsid protein of Brome mosaic virus using Bimolecular Fluorescence Complementation: implications for replication and genome packaging.

    Science.gov (United States)

    Chaturvedi, Sonali; Rao, A L N

    2014-09-01

    In Brome mosaic virus, it was hypothesized that a physical interaction between viral replicase and capsid protein (CP) is obligatory to confer genome packaging specificity. Here we tested this hypothesis by employing Bimolecular Fluorescent Complementation (BiFC) as a tool for evaluating protein-protein interactions in living cells. The efficacy of BiFC was validated by a known interaction between replicase protein 1a (p1a) and protein 2a (p2a) at the endoplasmic reticulum (ER) site of viral replication. Additionally, co-expression in planta of a bona fide pair of interacting protein partners of p1a and p2a had resulted in the assembly of a functional replicase. Subsequent BiFC assays in conjunction with mCherry labeled ER as a fluorescent cellular marker revealed that CP physically interacts with p2a, but not p1a, and this CP:p2a interaction occurs at the cytoplasmic phase of the ER. The significance of the CP:p2a interaction in BMV replication and genome packaging is discussed. Copyright © 2014 Elsevier Inc. All rights reserved.

  18. Vacancy-induced initial decomposition of condensed phase NTO via bimolecular hydrogen transfer mechanisms at high pressure: a DFT-D study.

    Science.gov (United States)

    Liu, Zhichao; Wu, Qiong; Zhu, Weihua; Xiao, Heming

    2015-04-28

    Density functional theory with dispersion-correction (DFT-D) was employed to study the effects of vacancy and pressure on the structure and initial decomposition of crystalline 5-nitro-2,4-dihydro-3H-1,2,4-triazol-3-one (β-NTO), a high-energy insensitive explosive. A comparative analysis of the chemical behaviors of NTO in the ideal bulk crystal and vacancy-containing crystals under applied hydrostatic compression was considered. Our calculated formation energy, vacancy interaction energy, electron density difference, and frontier orbitals reveal that the stability of NTO can be effectively manipulated by changing the molecular environment. Bimolecular hydrogen transfer is suggested to be a potential initial chemical reaction in the vacancy-containing NTO solid at 50 GPa, which is prior to the C-NO2 bond dissociation as its initiation decomposition in the gas phase. The vacancy defects introduced into the ideal bulk NTO crystal can produce a localized site, where the initiation decomposition is preferentially accelerated and then promotes further decompositions. Our results may shed some light on the influence of the molecular environments on the initial pathways in molecular explosives.

  19. Live cell imaging of interactions between replicase and capsid protein of Brome mosaic virus using Bimolecular Fluorescence Complementation: Implications for replication and genome packaging

    Energy Technology Data Exchange (ETDEWEB)

    Chaturvedi, Sonali; Rao, A.L.N., E-mail: arao@ucr.edu

    2014-09-15

    In Brome mosaic virus, it was hypothesized that a physical interaction between viral replicase and capsid protein (CP) is obligatory to confer genome packaging specificity. Here we tested this hypothesis by employing Bimolecular Fluorescent Complementation (BiFC) as a tool for evaluating protein–protein interactions in living cells. The efficacy of BiFC was validated by a known interaction between replicase protein 1a (p1a) and protein 2a (p2a) at the endoplasmic reticulum (ER) site of viral replication. Additionally, co-expression in planta of a bona fide pair of interacting protein partners of p1a and p2a had resulted in the assembly of a functional replicase. Subsequent BiFC assays in conjunction with mCherry labeled ER as a fluorescent cellular marker revealed that CP physically interacts with p2a, but not p1a, and this CP:p2a interaction occurs at the cytoplasmic phase of the ER. The significance of the CP:p2a interaction in BMV replication and genome packaging is discussed. - Highlights: • YFP fusion proteins of BMV p1a and p2a are biologically active. • Self-interaction was observed for p1a, p2a and CP. • CP interacts with p2a but not p1a. • Majority of reconstituted YFP resulting from bona fide fusion protein partners localized on ER.

  20. Live cell imaging of interactions between replicase and capsid protein of Brome mosaic virus using Bimolecular Fluorescence Complementation: Implications for replication and genome packaging

    International Nuclear Information System (INIS)

    Chaturvedi, Sonali; Rao, A.L.N.

    2014-01-01

    In Brome mosaic virus, it was hypothesized that a physical interaction between viral replicase and capsid protein (CP) is obligatory to confer genome packaging specificity. Here we tested this hypothesis by employing Bimolecular Fluorescent Complementation (BiFC) as a tool for evaluating protein–protein interactions in living cells. The efficacy of BiFC was validated by a known interaction between replicase protein 1a (p1a) and protein 2a (p2a) at the endoplasmic reticulum (ER) site of viral replication. Additionally, co-expression in planta of a bona fide pair of interacting protein partners of p1a and p2a had resulted in the assembly of a functional replicase. Subsequent BiFC assays in conjunction with mCherry labeled ER as a fluorescent cellular marker revealed that CP physically interacts with p2a, but not p1a, and this CP:p2a interaction occurs at the cytoplasmic phase of the ER. The significance of the CP:p2a interaction in BMV replication and genome packaging is discussed. - Highlights: • YFP fusion proteins of BMV p1a and p2a are biologically active. • Self-interaction was observed for p1a, p2a and CP. • CP interacts with p2a but not p1a. • Majority of reconstituted YFP resulting from bona fide fusion protein partners localized on ER

  1. Bimolecular interaction of argpyrimidine (a Maillard reaction product) in in vitro non-enzymatic protein glycation model and its potential role as an antiglycating agent.

    Science.gov (United States)

    Bhattacherjee, Abhishek; Dhara, Kaliprasanna; Chakraborti, Abhay Sankar

    2017-09-01

    Non- enzymatic glycation, also known as Maillard reaction, is one of the most important and investigated reactions in biochemistry. Maillard reaction products (MRPs) like protein-derived advanced glycation end products (AGEs) are often referred to cause pathophysiological complications in human systems. On contrary, several MRPs are exogenously used as antioxidant, antimicrobial and flavouring agents. In the preset study, we have shown that argpyrimidine, a well-established AGE, interacts with bovine serum albumin (BSA) and glucose individually in standard BSA-glucose model system and successfully inhibits glycation of the protein. Bimolecular interaction of argpyrimidine with glucose or BSA has been studied independently. Chromatographic purification, different spectroscopic studies and molecular modeling have been used to evaluate the nature and pattern of interactions. Binding of argpyrimidine with BSA prevents incorporation of glucose inside the native protein. Argpyrimidine can also directly entrap glucose. Both these interactions may be associated with the antiglycation potential of argpyrimidine, indicating a beneficial function of an AGE. Copyright © 2017 Elsevier B.V. All rights reserved.

  2. A mathematical analysis of Prx2-STAT3 disulfide exchange rate constants for a bimolecular reaction mechanism.

    Science.gov (United States)

    Langford, Troy F; Deen, William M; Sikes, Hadley D

    2018-03-22

    Appreciation of peroxiredoxins as the major regulators of H 2 O 2 concentrations in human cells has led to a new understanding of redox signaling. In addition to their status as the primary reducers of H 2 O 2 to water, the oxidized peroxiredoxin byproduct of this reaction has recently been shown capable of participation in H 2 O 2 -mediated signaling pathways through disulfide exchange reactions with the transcription factor STAT3. The dynamics of peroxidase-transcription factor disulfide exchange reactions have not yet been considered in detail with respect to how these reactions fit into the larger network of competing reactions in human cells. In this study, we used a kinetic model of oxidation and reduction reactions related to H 2 O 2 metabolism in the cytosol of human cells to study the dynamics of peroxiredoxin-2 mediated oxidation of the redox-regulated transcription factor STAT3. In combination with previously reported experimental data, the model was used to estimate the rate coefficient of a biomolecular reaction between Prx2 and STAT3 for two sets of assumptions that constitute lower and upper bound cases. Using these estimates, we calculated the relative rates of the reaction of oxidized peroxiredoxin-2 and STAT3 and other competing reactions in the cytosol. These calculations revealed that peroxiredoxin-2-mediated oxidation of STAT3 likely occurs at a much slower rate than competing reactions in the cytosol. This analysis suggests the existence of more complex mechanisms, potentially involving currently unknown protein-protein recognition partners, which facilitate disulfide exchange reactions between peroxiredoxin-2 and STAT3. Copyright © 2018 Elsevier Inc. All rights reserved.

  3. Observational Constraints of 30–40 GeV Dark Matter Annihilation in Galaxy Clusters

    Directory of Open Access Journals (Sweden)

    Man Ho Chan

    2016-01-01

    Full Text Available Recently, it has been shown that the annihilation of 30–40 GeV dark matter particles through bb- channel can satisfactorily explain the excess GeV gamma-ray spectrum near the Galactic Center. In this paper, we apply the above model to galaxy clusters and use the latest upper limits of gamma-ray flux derived from Fermi-LAT data to obtain an upper bound of the annihilation cross section of dark matter. By considering the extended density profiles and the cosmic ray profile models of 49 galaxy clusters, the upper bound of the annihilation cross section can be further tightened to σv≤9×10-26 cm3 s−1. This result is consistent with the one obtained from the data near the Galactic Center.

  4. Development of positron annihilation spectroscopy to test accelerated weathering of protective polymer coatings

    CERN Document Server

    Zhang, R; Chen, H M; Mallon, P; Sandreczki, T C; Richardson, J R; Jean, Y C; Nielsen, B; Suzuki, R; Ohdaira, T

    2000-01-01

    A variable mono-energetic positron beam with a computer-controlled system has recently been constructed at the University of Missouri-Kansas City for weathering studies of polymeric coatings. The beam is designed to measure the S-parameter from Doppler-broadening energy spectra and the sub-nanometer defect properties from positron annihilation lifetimes (PAL). Significant variations of S-parameter and ortho-positronium intensity in coatings, as obtained from the newly built beam and from the Electrotechnical Laboratory's beam, respectively, are observed as a function of depth and exposure time due to the Xe-light irradiation. A high sensitivity of positron annihilation signal response to the early stage of degradation is observed. Development of positron annihilation spectroscopy to test accelerated weathering of polymeric coatings is discussed.

  5. Investigation of silicon sensors for their use as antiproton annihilation detectors

    Energy Technology Data Exchange (ETDEWEB)

    Pacifico, N., E-mail: nicola.pacifico@cern.ch [University of Bergen, Institute of Physics and Technology, Allégaten 55, 5007 Bergen (Norway); Aghion, S. [Politecnico di Milano, Piazza Leonardo da Vinci 32, 20133 Milano (Italy); Istituto Nazionale di Fisica Nucleare, Sez. di Milano, Via Celoria 16, 20133 Milano (Italy); Ahlén, O. [European Organisation for Nuclear Research, Physics Department, 1211 Geneva 23 (Switzerland); Belov, A.S. [Institute for Nuclear Research of the Russian Academy of Sciences, Moscow 117312 (Russian Federation); Bonomi, G. [University of Brescia, Department of Mechanical and Industrial Engineering, Via Branze 38, 25133 Brescia (Italy); Istituto Nazionale di Fisica Nucleare, Sez. di Pavia, Via Agostino Bassi 6, 27100 Pavia (Italy); Bräunig, P. [Kirchhoff Institute for Physics, Im Neuenheimer Feld 227, 69120 Heidelberg (Germany); Bremer, J. [European Organisation for Nuclear Research, Physics Department, 1211 Geneva 23 (Switzerland); Brusa, R.S. [Department of Physics, University of Trento, via Sommarive 14, 38123 Povo, Trento (Italy); INFN-TIFPA, via Sommarive 14, 38123 Povo, Trento (Italy); Burghart, G. [European Organisation for Nuclear Research, Physics Department, 1211 Geneva 23 (Switzerland); Cabaret, L. [Laboratoire Aimé Cotton, CNRS, Université Paris Sud, ENS Cachan, Bâtiment 505, Campus d' Orsay, 91405 Orsay Cedex (France); Caccia, M. [University of Insubria, Dipartimento di Scienza ed Alta Tecnologia, via Valleggio 11, Como (Italy); Canali, C. [University of Zurich, Physics Institute, Winterthurerstrasse 190, 8057 Zurich (Switzerland); Caravita, R. [Istituto Nazionale di Fisica Nucleare, Sez. di Genova, Via Dodecaneso 33, 16146 Genova (Italy); University of Genoa, Department of Physics, Via Dodecaneso 33, 16146 Genova (Italy); Castelli, F. [University of Milano, Department of Physics, Via Celoria 16, 20133 Milano (Italy); and others

    2014-11-21

    We present here a new application of silicon sensors aimed at the direct detection of antinucleons annihilations taking place inside the sensor's volume. Such detectors are interesting particularly for the measurement of antimatter properties and will be used as part of the gravity measurement module in the AEg{sup ¯}IS experiment at the CERN Antiproton Decelerator. One of the goals of the AEg{sup ¯}IS experiment is to measure the gravitational acceleration of antihydrogen with 1% precision. Three different silicon sensor geometries have been tested with an antiproton beam to investigate their properties as annihilation detection devices: strip planar, 3D pixels and monolithic pixel planar. In all cases we were successfully detecting annihilations taking place in the sensor and we were able to make a first characterization of the clusters and tracks.

  6. Surface investigations by means of positrons annihilation; Badania warstwy wierzchniej metoda anihilacji pozytonow

    Energy Technology Data Exchange (ETDEWEB)

    Dryzek, J. [Institute of Nuclear Physics, Cracow (Poland); Stegemann, T.; Cleff, B. [Muenster Univ. (Germany). Inst. fuer Kernphysik

    1996-12-31

    The aim of the report is a presentation of the positron annihilation studies performed on the Cu samples that surface was exposed to the friction and wear processes. Using the measurement of Doppler broadening of annihilation line, we were able to detect the profile of vacancies in the top layers of the defected metals. It was established that one could describe the profile by a simple exponential function of the depth in all cases. The range of vacancies concentration depth depends on the load, time and the speed of the defects creation processes on the surface of a sample. The outline of the positron annihilation method is also given. (author). 10 refs, 16 figs, 5 tabs.

  7. Evidence of mesoniums in anti pn annihilations and γγ reactions

    International Nuclear Information System (INIS)

    Liu, K.F.; Li, B.A.

    1987-01-01

    A new resonance at 1480 MeV with a width of 110 MeV is found in anti pn annihilations in the channel anti pn → π - X 0 (1480) → π - ρ 0 ρ 0 . Its mass, width and spin-parity are shown to be consistent with the ρ 0 ρ 0 enhancement observed in γγ reactions. Together with the suppression in the γγ → ρ + ρ - data which requires the admixture of an isotensor structure, this ρ 0 ρ 0 resonance in anti pn annihilation and γγ reactions and their small ππ branching ratios represent the best evidence yet for the Q 2 Q-bar 2 nature of the mesoniums. A ρ - ρ - resonance in anti pn annihilations which would betray the exotic isotensor nature of the resonance is predicted. (author)

  8. Neutralino-stop co-annihilation into electroweak gauge and Higgs bosons at one loop

    Energy Technology Data Exchange (ETDEWEB)

    Harz, J. [Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Herrmann, B. [Univ. Savoie/CNRS, Annecy-le-Vieux (France). LAPTh; Klasen, M. [Muenster Univ. (Germany). Inst. fuer Theoretische Physik 1; Kovarik, K. [Karlsruhe Institute of Technology, Karlsruhe (Germany). Inst. for Theoretical Physics; Le Boulc' h, Q. [Grenoble Univ. (France). CNRS-IN2P3/INPG

    2012-12-15

    We compute the full O({alpha}{sub s}) supersymmetric QCD corrections for neutralino-stop co-annihilation into electroweak gauge and Higgs bosons in the Minimal Supersymmetric Standard Model (MSSM). We show that these annihilation channels are phenomenologically relevant within the so-called phenomenological MSSM, in particular in the light of the observation of a Higgs-like particle with a mass of about 126 GeV at the LHC. We present in detail our calculation, including the renormalization scheme, the infrared treatment, and the kinematical subtleties to be addressed. Numerical results for the co-annihilation cross sections and the predicted neutralino relic density are presented. We demonstrate that the impact of including the corrections on the cosmologically preferred region of parameter space is larger than the current experimental uncertainty from WMAP data.

  9. Diffuse gamma ray constraints on annihilating or decaying Dark Matter after Fermi

    International Nuclear Information System (INIS)

    Cirelli, Marco; Panci, Paolo; Serpico, Pasquale D.

    2010-01-01

    We consider the diffuse gamma ray data from Fermi first year observations and compare them to the gamma ray fluxes predicted by Dark Matter annihilation or decay (both from prompt emission and from Inverse Compton Scattering), for different observation regions of the sky and a range of Dark Matter masses, annihilation/decay channels and Dark Matter galactic profiles. We find that the data exclude large regions of the Dark Matter parameter space not constrained otherwise and discuss possible directions for future improvements. Also, we further constrain Dark Matter interpretations of the e ± PAMELA/Fermi spectral anomalies, both for the annihilating and the decaying Dark Matter case: under very conservative assumptions, only models producing dominantly μ ± and assuming a cored Dark Matter galactic profile can fit the lepton data with masses around ∼2 TeV.

  10. Stop co-annihilation in the minimal supersymmetric standard model revisited

    Science.gov (United States)

    Pierce, Aaron; Shah, Nausheen R.; Vogl, Stefan

    2018-01-01

    We reexamine the stop co-annihilation scenario of the minimal supersymmetric standard model, wherein a binolike lightest supersymmetric particle has a thermal relic density set by co-annihilations with a scalar partner of the top quark in the early universe. We concentrate on the case where only the top partner sector is relevant for the cosmology, and other particles are heavy. We discuss the cosmology with focus on low energy parameters and an emphasis on the implications of the measured Higgs boson mass and its properties. We find that the irreducible direct detection signal correlated with this cosmology is generically well below projected experimental sensitivity, and in most cases lies below the neutrino background. A larger, detectable, direct detection rate is possible, but is unrelated to the co-annihilation cosmology. LHC searches for compressed spectra are crucial for probing this scenario.

  11. Non-standard interactions and neutrinos from dark matter annihilation in the Sun

    Science.gov (United States)

    Demidov, S. V.

    2018-02-01

    We perform an analysis of the influence of non-standard neutrino interactions (NSI) on neutrino signal from dark matter annihilations in the Sun. Taking experimentally allowed benchmark values for the matter NSI parameters we show that the evolution of such neutrinos with energies at GeV scale can be considerably modified. We simulate propagation of neutrinos from the Sun to the Earth for realistic dark matter annihilation channels and find that the matter NSI can result in at most 30% correction to the signal rate of muon track events at neutrino telescopes. Still present experimental bounds on dark matter from these searches are robust in the presence of NSI within considerable part of their allowed parameter space. At the same time electron neutrino flux from dark matter annihilation in the Sun can be changed by a factor of few.

  12. The annihilation of positrons in the cold phase of the interstellar medium revisited

    Science.gov (United States)

    Wallyn, P.; Durouchoux, PH.; Chapuis, C.; Leventhal, M.

    1994-01-01

    The positron cross sections in H and H2 media are reevaluated, taking into account new experimental results. Using a Monte Carlo simulation, we find a positronium fraction before thermalization of 0.90 for H2, in good agreement with the previous experimental result given by Brown et al. (1986). For H we obtain an upper limit of 0.98. We study the behavior of the charge exchange annihilation in a cold phase (molecular cloud). We calculate a formula for the slowing-down time t, before annihilation lasting Delta t, via charge exchange, of a positron beam with a given energy for different medium densities and initial energies. An upper limit of 0.7 MeV for the initial energy of the positrons, annihilating in the molecular cloud G0.86 - 0.08 near the gamma ray source positronium and gives new time constraints on their possible observation.

  13. Positron annihilation in pivalic acid. Temperature dependence of angular correlation curves

    DEFF Research Database (Denmark)

    Jain, P. C.; Eldrup, Morten Mostgaard; Pedersen, Niels Jørgen

    1986-01-01

    Positron annihilation angular correlation curves have been measured as a function of temperature for trimethylacetic (pivalic) acid in both the brittle and plastic phases. A simple fitting of the data to a sum of three gaussians shows the presence of a narrow component due to para-positronium (p......-Ps) annihilation. In the brittle phase the intensity of the narrow component is inconsistent with previous positron lifetime data. A more detailed analysis, requiring consistency with the lifetime data, results in the determination of the shapes of the angular correlation components for free positron-, pick......-off-, and p-Ps intrinsic annihilation. The p-Ps component has a width (fwhm) of 3.75 mrad in the brittle phase, probably due to Ps self-trapping or trapping in defects smaller than molecular vacancies. In the plastic phase the width (fwhm) is 3.25 mrad which is ascribed to Ps localization in vacancies...

  14. Nanoscopic properties of silica filled polydimethylsiloxane by means of positron annihilation lifetime spectroscopy

    DEFF Research Database (Denmark)

    Wiinberg, P.; Eldrup, Morten Mostgaard; Maurer, F.H.J.

    2004-01-01

    Positron annihilation lifetime spectroscopy (PALS) was performed on a series of polydimethylsiloxane (PDMS)/fumed silicon dioxide (SiO2) composites at temperatures between -185 and 100degreesC to study the effect of filler content and filler particle size on the free volume properties and the pos......Positron annihilation lifetime spectroscopy (PALS) was performed on a series of polydimethylsiloxane (PDMS)/fumed silicon dioxide (SiO2) composites at temperatures between -185 and 100degreesC to study the effect of filler content and filler particle size on the free volume properties...... and the positron annihilation characteristics. The glass transition behavior of the PDMS/SiO2 composites was determined with differential scanning calorimetry. A clear influence on the o-Ps lifetime (73) in the polymer upon addition of nano-sized fumed SiO2 was observed at all temperatures. The observed o...

  15. Early Stages of Precipitation Process in Al-(Mn-)Sc-Zr Alloy Characterized by Positron Annihilation

    KAUST Repository

    Vlach, Martin

    2015-01-29

    Thermal effects on the precipitation stages in as-cast Al-0.70 at. pct Mn-0.15 at. pct Sc-0.05 at. pct Zr alloy were studied. The role of lattice defects was elucidated by positron annihilation spectroscopy (lifetime and coincidence Doppler broadening) enabling investigation of solutes clustering at the atomic scale. This technique has never been used in the Al-Sc- and/or Al-Zr-based alloys so far. Studies by positron annihilation were combined with resistometry, hardness measurements, and microstructure observations. Positrons trapped at defects are preferentially annihilated by Sc electrons. Lifetime of trapped positrons indicates that Sc atoms segregate at dislocations. Maximum fraction of positrons annihilated by Sc electrons occurring at 453 K (180 °C) suggests that clustering of Sc bound with vacancies takes place. It is followed by peak of this fraction at 573 K (300 °C). A rise of the contribution of trapped positrons annihilated by Zr electrons starting at 513 K (240 °C) and attaining maximum also at 573 K (300 °C) confirms that Zr participates in precipitation of the Al3Sc particles already at these temperatures. The pronounced hardening at 573 K (300 °C) has its nature in the precipitation of the Al3Sc particles with a Zr-rich shell. The contribution of trapped positrons annihilated by Mn electrons was found to be negligible. © 2015, The Minerals, Metals & Materials Society and ASM International.

  16. On the Sunyaev-Zel'dovich effect from dark matter annihilation or decay in galaxy clusters

    International Nuclear Information System (INIS)

    Lavalle, Julien; Boehm, Céline; Barthès, Julien

    2010-01-01

    We revisit the prospects for detecting the Sunyaev Zel'dovich (SZ) effect induced by dark matter (DM) annihilation or decay. We show that with standard (or even extreme) assumptions for DM properties, the optical depth associated with relativistic electrons injected from DM annihilation or decay is much smaller than that associated with thermal electrons, when averaged over the angular resolution of current and future experiments. For example, we find: τ DM ∼ 10 −9 −10 −5 (depending on the assumptions) for m χ = 1 GeV and a density profile ρ∝r −1 for a template cluster located at 50 Mpc and observed within an angular resolution of 10'', compared to τ th ∼ 10 −3 −10 −2 . This, together with a full spectral analysis, enables us to demonstrate that, for a template cluster with generic properties, the SZ effect due to DM annihilation or decay is far below the sensitivity of the Planck satellite. This is at variance with previous claims regarding heavier annihilating DM particles. Should DM be made of lighter particles, the current constraints from 511 keV observations on the annihilation cross section or decay rate still prevent a detectable SZ effect. Finally, we show that spatial diffusion sets a core of a few kpc in the electron distribution, even for very cuspy DM profiles, such that improving the angular resolution of the instrument, eg with ALMA, does not necessarily improve the detection potential. We provide useful analytical formulæ parameterized in terms of the DM mass, decay rate or annihilation cross section and DM halo features, that allow quick estimates of the SZ effect induced by any given candidate and any DM halo profile

  17. Measurement of positron annihilation lifetimes for positron burst by multi-detector array

    Science.gov (United States)

    Wang, B. Y.; Kuang, P.; Liu, F. Y.; Han, Z. J.; Cao, X. Z.; Zhang, P.

    2018-03-01

    It is currently impossible to exploit the timing information in a gamma-ray pulse generated within nanoseconds when a high-intensity positron burst annihilation event occurs in a target using conventional single-detector methods. A state-of-the-art solution to the problem is proposed in this paper. In this approach, a multi-detector array composed of many independent detection cells mounted spherically around the target is designed to detect the time distribution of the annihilated gamma rays generated following, in particular, a positron burst emitting huge amounts of positrons in a short pulse duration, even less than a few nano- or picoseconds.

  18. Determination of the solubility of neodymium in iron by positron annihilation

    International Nuclear Information System (INIS)

    Yu, W.Y.; Qing, L.N.; Zhuo, T.Z.; Rong, C.X.

    1985-01-01

    The authors have measured the lineshape parameters and lifetimes of positron annihilation in eleven samples of iron containing various concentration of Nd between 0 and 0.87 wt. %, which have been heat-treated at two different temperatures successively. According to the abrupt increase, for the two conditions of heat-treatment the solubility of Nd in iron is interpreted to be 0.082 wt. % and 0.088 wt. % respectively. Using positron annihilation technique for determining the solubility of Nd in iron appears to be more sensitive and accurate than metallography method and X-ray diffraction analysis

  19. Positron annihilation in pivalic acid. Temperature dependence of angular correlation curves

    DEFF Research Database (Denmark)

    Jain, P. C.; Eldrup, Morten Mostgaard; Pedersen, Niels Jørgen

    1986-01-01

    -off-, and p-Ps intrinsic annihilation. The p-Ps component has a width (fwhm) of 3.75 mrad in the brittle phase, probably due to Ps self-trapping or trapping in defects smaller than molecular vacancies. In the plastic phase the width (fwhm) is 3.25 mrad which is ascribed to Ps localization in vacancies......Positron annihilation angular correlation curves have been measured as a function of temperature for trimethylacetic (pivalic) acid in both the brittle and plastic phases. A simple fitting of the data to a sum of three gaussians shows the presence of a narrow component due to para-positronium (p...

  20. How to distinguish between the annihilation and the creation of optical vortices

    CSIR Research Space (South Africa)

    Roux, FS

    2013-10-01

    Full Text Available been cre- ated, we start with a simple illustrative example. The analyses of second-order polynomial Gaussian beams [18, 19] allow one to construct examples of beams con- taining vortex dipoles that will either be annihilated or created in the waist... and annihilation events. Cre- ations always appear in positive regions and annihila- tions always appear in negative regions. Due to the continuity of the vitality in Eq. (10) as a function in three dimensions, we extended the iden- tification of the event at a...

  1. Positron-annihilation 2D-ACAR studies of disordered and defected alloys

    International Nuclear Information System (INIS)

    Bansil, A.; Prasad, R.; Smedskjaer, L.C.; Benedek, R.; Mijnarends, P.E.

    1987-09-01

    Theoretical and experimental progess in connection with 2D-ACAR positron annihilation studies of ordered, disordered, and defected alloys is discussed. We present, in particular, some of the recent developments concerning the electronic structure of disordered alloys, and the work in the area of annihilation from positrons trapped at vacancy-type defects in metals and alloys. The electronic structure and properties of a number of compounds are also discussed briefly; we comment specifically on high T/sub c/ ceramic superconductors, Heusler alloys, and transition-metal aluminides. 58 refs., 116 figs

  2. Positron annihilation studies of mesoporous silica films using a slow positron beam

    International Nuclear Information System (INIS)

    He Chunqing; Muramatsu, Makoto; Ohdaira, Toshiyuki; Kinomura, Atsushi; Suzuki, Ryoichi; Ito, Kenji; Kabayashi, Yoshinori

    2006-01-01

    Positron annihilation lifetime spectra were measured for mesoporous silica films, which were synthesized using triblock copolymer (EO 106 PO 70 EO 106 ) as a structure-directing agent. Different positron lifetime spectra for the deposited and calcined films indicated the formation of meso-structure after calcination, which was confirmed by Fourier transform infrared (FTIR) spectra and field emission-scanning electron microscopy (FE-SEM) observation. Open porosity or pore interconnectivity of a silica film might be evaluated by a two-dimensional positron annihilation lifetime spectrum of an uncapped film. Pore sizes and their distributions in the silica films were found to be affected by thermal treatments

  3. Studies of Phase Transformation in Molecular Crystals Using the Positron Annihilation Technique

    DEFF Research Database (Denmark)

    Eldrup, Morten Mostgaard; Lightbody, David; Sherwood, John N.

    1980-01-01

    An examination has been made of the brittle/plastic phase transformation in the molecular crystals cyclohexane, DL-camphene and succinonitrile using the positron annihilation technique. In each material, the transition is characterized by a distinct increase in ortho-positronium lifetime. The inf......An examination has been made of the brittle/plastic phase transformation in the molecular crystals cyclohexane, DL-camphene and succinonitrile using the positron annihilation technique. In each material, the transition is characterized by a distinct increase in ortho-positronium lifetime...

  4. Cascade sensitization of triplet-triplet annihilation based photon upconversion at sub-solar irradiance.

    Science.gov (United States)

    Pedrini, Jacopo; Monguzzi, Angelo; Meinardi, Francesco

    2018-04-03

    In triplet-triplet annihilation based upconversion, high-energy photons are generated through the annihilation of fluorophore triplets, populated via energy transfer from a light-harvesting sensitizer. However, the absorption band of common sensitizers is narrow, limiting the fraction of recoverable photons. We overcome this issue using a third chromophore as an additional light-harvester in the transparency window between the upconverted luminescence and the sensitizer absorption. The third component transfers the extra-collected energy to sensitizers, realizing a cascade-sensitized upconversion that shows a 20% increment of the high-energy photon output and a conversion yield of 10% at solar irradiance.

  5. Temperature Dependence of Triplet–Triplet Annihilation Upconversion in Phospholipid Membranes

    Science.gov (United States)

    2017-01-01

    Understanding the temperature dependency of triplet–triplet annihilation upconversion (TTA-UC) is important for optimizing biological applications of upconversion. Here the temperature dependency of red-to-blue TTA-UC is reported in a variety of neutral PEGylated phospholipid liposomes. In these systems a delicate balance between lateral diffusion rate of the dyes, annihilator aggregation, and sensitizer self-quenching leads to a volcano plot, with the maximum upconversion intensity occurring near the main order–disorder transition temperature of the lipid membrane. PMID:28059523

  6. Charmed Mesons Produced in e+e- Annihilation

    Energy Technology Data Exchange (ETDEWEB)

    Goldhaber, G.; Wiss, J. E.

    1980-12-01

    We shall begin our review by summarizing the first experimental indications for the existence of charm as obtained from experiments in e{sup +}e{sup -} annihilation. This will include a brief discussion of the role of charm in the understanding of the {psi} mesons, as well as the unraveling of the intricate structure present in the e{sup +} e{sup -} total hadronic cross section. Next we shall discuss the discovery of the D{sup 0}, and D{sup +}, and detail those properties crucial to their identification as charmed particles. Following will be a review of the properties of the D{sup 0} and D{sup +} learned through studies at the {psi}(3770) resonance, Compelling evidence will be summarized indicating that this state decays nearly exclusively into D{bar D}, thus making it particularly useful in establishing inclusive and exclusive D branching fractions. Our discussion of branching fractions will include two particularly important D decay modes, D{sup 0}{yields}{pi}{sup +}{pi}{sup -} and D{sup 0}{yields}K{sup +}{sup -}. These processes are suppressed relative to D{sup 0}{yields}K{sup -}{pi}{sup +} in the standard charm model, and thus serve as a critical test of that theory. This will be followed by a discussion of the D semileptonic decay modes which provide useful information on the D{sup 0} and D{sup +} lifetimes. Turning our attention to the data collected beyond the {psi}(3770) we will discuss the properties and production mechanisms of the excited charm mesons, the D*{sup 0} and the D*{sup +}. D production just above the {psi}(3770) appears to be dominated by the three quasi-two-body processes e{sup +} e{sup -} {yields} D{bar D}, D*{bar D} + {bar D}*D, and D*{bar D}*, in accordance with early theoretical predictions. The relative amounts of each process, on the other hand, is somewhat surprising, and has led to considerable theoretical speculation. Finally, we will summarize evidence for the existence of the F meson which is as yet not on as solid a footing as

  7. Exciton-Exciton Annihilation Is Coherently Suppressed in H-Aggregates, but Not in J-Aggregates.

    Science.gov (United States)

    Tempelaar, Roel; Jansen, Thomas L C; Knoester, Jasper

    2017-12-21

    We theoretically demonstrate a strong dependence of the annihilation rate between (singlet) excitons on the sign of dipole-dipole couplings between molecules. For molecular H-aggregates, where this sign is positive, the phase relation of the delocalized two-exciton wave functions causes a destructive interference in the annihilation probability. For J-aggregates, where this sign is negative, the interference is constructive instead; as a result, no such coherent suppression of the annihilation rate occurs. As a consequence, room temperature annihilation rates of typical H- and J-aggregates differ by a factor of ∼3, while an order of magnitude difference is found for low-temperature aggregates with a low degree of disorder. These findings, which explain experimental observations, reveal a fundamental principle underlying exciton-exciton annihilation, with major implications for technological devices and experimental studies involving high excitation densities.

  8. Exciton–Exciton Annihilation Is Coherently Suppressed in H-Aggregates, but Not in J-Aggregates

    Science.gov (United States)

    2017-01-01

    We theoretically demonstrate a strong dependence of the annihilation rate between (singlet) excitons on the sign of dipole–dipole couplings between molecules. For molecular H-aggregates, where this sign is positive, the phase relation of the delocalized two-exciton wave functions causes a destructive interference in the annihilation probability. For J-aggregates, where this sign is negative, the interference is constructive instead; as a result, no such coherent suppression of the annihilation rate occurs. As a consequence, room temperature annihilation rates of typical H- and J-aggregates differ by a factor of ∼3, while an order of magnitude difference is found for low-temperature aggregates with a low degree of disorder. These findings, which explain experimental observations, reveal a fundamental principle underlying exciton–exciton annihilation, with major implications for technological devices and experimental studies involving high excitation densities. PMID:29190421

  9. Perspective: chemical dynamics simulations of non-statistical reaction dynamics.

    Science.gov (United States)

    Ma, Xinyou; Hase, William L

    2017-04-28

    Non-statistical chemical dynamics are exemplified by disagreements with the transition state (TS), RRKM and phase space theories of chemical kinetics and dynamics. The intrinsic reaction coordinate (IRC) is often used for the former two theories, and non-statistical dynamics arising from non-IRC dynamics are often important. In this perspective, non-statistical dynamics are discussed for chemical reactions, with results primarily obtained from chemical dynamics simulations and to a lesser extent from experiment. The non-statistical dynamical properties discussed are: post-TS dynamics, including potential energy surface bifurcations, product energy partitioning in unimolecular dissociation and avoiding exit-channel potential energy minima; non-RRKM unimolecular decomposition; non-IRC dynamics; direct mechanisms for bimolecular reactions with pre- and/or post-reaction potential energy minima; non-TS theory barrier recrossings; and roaming dynamics.This article is part of the themed issue 'Theoretical and computational studies of non-equilibrium and non-statistical dynamics in the gas phase, in the condensed phase and at interfaces'. © 2017 The Author(s).

  10. Dynamics

    CERN Document Server

    Goodman, Lawrence E

    2001-01-01

    Beginning text presents complete theoretical treatment of mechanical model systems and deals with technological applications. Topics include introduction to calculus of vectors, particle motion, dynamics of particle systems and plane rigid bodies, technical applications in plane motions, theory of mechanical vibrations, and more. Exercises and answers appear in each chapter.

  11. SUSY-QCD corrections to the (co)annihilation of neutralino dark matter within the MSSM

    Energy Technology Data Exchange (ETDEWEB)

    Meinecke, Moritz

    2015-06-15

    Based on experimental observations, it is nowadays assumed that a large component of the matter content in the universe is comprised of so-called cold dark matter. Furthermore, latest measurements of the temperature fluctuations of the cosmic microwave background provided an estimation of the dark matter relic density at a measurement error of one percent (concerning the experimental 1σ-error). The lightest neutralino χ 0{sub 1}, a particle which subsumes under the phenomenologically interesting category of weakly interacting massive particles, is a viable dark matter candidate for many supersymmetric (SUSY) models whose relic density Ω{sub χ} {sub 0{sub 1}} happens to lie quite naturally within the experimentally favored ballpark of dark matter. The high experimental precision can be used to constrain the SUSY parameter space to its cosmologically favored regions and to pin down phenomenologically interesting scenarios. However, to actually benefit from this progress on the experimental side it is also mandatory to minimize the theoretical uncertainties. An important quantity within the calculation of the neutralino relic density is the thermally averaged sum over different annihilation and coannihilation cross sections of the neutralino and further supersymmetric particles. It is now assumed and also partly proven that these cross sections can be subject to large loop corrections which can even shift the associated Ω{sub χ} {sub 0{sub 1}} by a factor larger than the current experimental error. However, most of these corrections are yet unknown. In this thesis, we calculate higher-order corrections for some of the most important (co)annihilation channels both within the framework of the R-parity conserving Minimal Supersymmetric Standard Model (MSSM) and investigate their impact on the final neutralino relic density Ω{sub χ} {sub 0{sub 1}}. More precisely, this work provides the full O(α{sub s}) corrections of supersymmetric quantum chromodynamics (SUSY

  12. A fluorescent bimolecular complementation screen reveals MAF1, RNF7 and SETD3 as PCNA-associated proteins in human cells

    Science.gov (United States)

    Cooper, Simon E; Hodimont, Elsie; Green, Catherine M

    2015-01-01

    The proliferating cell nuclear antigen (PCNA) is a conserved component of DNA replication factories, and interactions with PCNA mediate the recruitment of many essential DNA replication enzymes to these sites of DNA synthesis. A complete description of the structure and composition of these factories remains elusive, and a better knowledge of them will improve our understanding of how the maintenance of genome and epigenetic stability is achieved. To fully characterize the set of proteins that interact with PCNA we developed a bimolecular fluorescence complementation (BiFC) screen for PCNA-interactors in human cells. This 2-hybrid type screen for interactors from a human cDNA library is rapid and efficient. The fluorescent read-out for protein interaction enables facile selection of interacting clones, and we combined this with next generation sequencing to identify the cDNAs encoding the interacting proteins. This method was able to reproducibly identify previously characterized PCNA-interactors but importantly also identified RNF7, Maf1 and SetD3 as PCNA-interacting proteins. We validated these interactions by co-immunoprecipitation from human cell extracts and by interaction analyses using recombinant proteins. These results show that the BiFC screen is a valuable method for the identification of protein-protein interactions in living mammalian cells. This approach has potentially wide application as it is high throughput and readily automated. We suggest that, given this interaction with PCNA, Maf1, RNF7, and SetD3 are potentially involved in DNA replication, DNA repair, or associated processes. PMID:26030842

  13. Experimental results on QCD [Quantum Chromodynamics] from e+e- annihilation

    International Nuclear Information System (INIS)

    de Boer, W.

    1987-09-01

    A review is given on QCD results from studying e + e - annihilation with the PEP and PETRA storage rings with special emphasis on jet physics and the determination of the strong coupling constant α/sub s/. 92 refs., 28 figs., 3 tabs

  14. Experimental results on QCD (Quantum Chromodynamics) from e/sup +/e/sup -/ annihilation

    Energy Technology Data Exchange (ETDEWEB)

    de Boer, W.

    1987-09-01

    A review is given on QCD results from studying e/sup +/e/sup -/ annihilation with the PEP and PETRA storage rings with special emphasis on jet physics and the determination of the strong coupling constant ..cap alpha../sub s/. 92 refs., 28 figs., 3 tabs.

  15. A study of Two Photon Decays of Charmonium Resonances Formed in Proton Anti-Proton Annihilations

    Energy Technology Data Exchange (ETDEWEB)

    Pedlar, Todd Kristofer [Northwestern Univ., Evanston, IL (United States)

    1999-06-01

    In this dissertation we describe the results of an investigation of the production of charmonium states (ηc, η'c, χ0 and χ2) in Fermilab experiment E835 via antiproton-proton annihilation and their detection via their decay into two photons.

  16. Limits on dark matter annihilation in the sun using the ANTARES neutrino telescope

    NARCIS (Netherlands)

    Adrián-Martínez, S.; Albert, A.; André, M.; Anton, G.; Ardid, M.; Aubert, J.-J.; Avgitas, T.; Baret, B.; Barrios-Martí, J.; Basa, S.; Bertin, V.; Biagi, S.; Bormuth, R.; Bouwhuis, M.C.; Bruijn, R.; Brunner, J.; Busto, J.; Capone, A.; Caramete, L.; Carr, J.; Celli, S.; Chiarusi, T.; Circella, M.; Coleiro, A.; Coniglione, R.; Costantini, H.; Coyle, P.; Creusot, A.; Deschamps, A.; De Bonis, G.; Distefano, C.; Donzaud, C.; Dornic, D.; Drouhin, D.; Eberl, T.; El Bojaddaini, I.; Elsässer, D.; Enzenhöfer, A.; Fehn, K.; Felis, I.; Fusco, L.A.; Galatà, S.; Gay, P.; Geißelsöder, S.; Geyer, K.; Giordano, V.; Gleixner, A.; Glotin, H.; Gracia-Ruiz, R.; Graf, K.; Hallmann, S.; van Haren, H.; Heijboer, A.J.; Hello, Y.; Hernández-Rey, J. J.; Hößl, J.; Hofestädt, J.; Hugon, C.; Illuminati, G.; James, C.W.; de Jong, M.; Jongen, M.; Kadler, M.; Kalekin, O.; Katz, U.; Kießling, D.; Kouchner, A.; Kreter, M.; Kreykenbohm, I.; Kulikovskiy, V.; Lachaud, C.; Lahmann, R.; Lefèvre, D.; Leonora, E.; Loucatos, S.; Marcelin, M.; Margiotta, A.; Marinelli, A.; Martínez-Mora, J.A.; Mathieu, A.; Melis, K.; Michael, T.; Migliozzi, P.; Moussa, A.; Mueller, C.; Nezri, E.; Păvălaş, G.E.; Pellegrino, C.; Perrina, C.; Piattelli, P.; Popa, V.; Pradier, T.; Racca, C.; Riccobene, G.; Roensch, K.; Saldaña, M.; Samtleben, D.F.E.; Sánchez-Losa, A.; Sanguineti, M.; Sapienza, P.; Schnabel, J.; Schüssler, F.; Seitz, T.; Sieger, C.; Spurio, M.; Stolarczyk, T.; Taiuti, M.; Tönnis, C.; Trovato, A.; Tselengidou, M.; Turpin, D.; Vallage, B.; Vallée, C.; Van Elewyck, V.; Vivolo, D.; Wagner, S.; Wilms, J.; Zornoza, J.D.; Zúñiga, J.

    A search for muon neutrinos originating from dark matter annihilations in the Sun is performed using the data recorded by the ANTARES neutrino telescope from 2007 to 2012. In order to obtain the best possible sensitivities to dark matter signals, an optimisation of the event selection criteria is

  17. Influence of mobility and annihilation of forest dislocations on radiation creep rate of metals

    International Nuclear Information System (INIS)

    Pyatiletov, Yu.S.; Tyupkina, O.G.

    1988-01-01

    Dependence of radiation creep rate ε of metals on stress σ is calculated. It is established that account of mobility and annihilation of 'forest' dislocations leads to the increase of calculational value ε and the effect increases with the growth of σ, reaching 10-15% at σ ∼ 0.8 σ cr (σ cr - critical shear stress)

  18. Scalar electron production in e/sup +/ e/sup -/ annihilation at high energies

    Energy Technology Data Exchange (ETDEWEB)

    Hayashibara, I.; Takasaki, F.; Shimizu, Y.; Kuroda, M.

    1985-08-22

    The cross section for single and pair productions of scalar electrons in e/sup +/e/sup -/ annihilation are calculated in the energy range of TRISTAN, SLC and LEP with specific emphasis on the contribution from the Z/sup 0/ boson and the zino. (orig.).

  19. Scalar electron production in e/sup +/ e annihilation at high energies

    Energy Technology Data Exchange (ETDEWEB)

    Hayashibara, I.; National Lab. for High Energy Physics, Tsukuba, Itabashi; Takasaki, F.; Shimizu, Y.; Kuroda, M.

    1985-08-22

    The cross section for single and pair productions of scalar electrons in e/sup +/e annihilation are calculated in the energy range of TRISTAN, SLC and LEP with specific emphasis on the contribution from the Z/sup 0/ boson and the zino. (orig.).

  20. Search for right-handed neutrinos from dark matter annihilation with gamma-rays

    International Nuclear Information System (INIS)

    Campos, Miguel D.; Queiroz, Farinaldo S.; Yaguna, Carlos E.; Weniger, Christoph

    2017-01-01

    Several extensions of the Standard Model contain right-handed (sterile) neutrinos in the GeV-TeV mass range. Due to their mixing with the active neutrinos, they may give rise to novel effects in cosmology, neutrino physics, and collider searches. In addition, right-handed neutrinos can also appear as final states from dark matter annihilations, with important implications for dark matter indirect detection searches. In this paper, we use current data from the Fermi Large Area Telescope (6-year observation of dwarf spheroidal galaxies) and H.E.S.S. (10-year observation of the Galactic center) to constrain the annihilation of dark matter into right-handed neutrinos. We consider right-handed neutrino with masses between 10 GeV and 1 TeV, including both two-body and three-body decays, to derive bounds on the dark matter annihilation rate, ( σ v ), as a function of the dark matter mass. Our results show, in particular, that the thermal dark matter annihilation cross section, 3× 10 −26 cm 3 s −1 , into right-handed neutrinos is excluded for dark matter masses smaller than 200 GeV.

  1. A survey of models of baryon production in e+e- annihilation

    International Nuclear Information System (INIS)

    Bell, K.W.; Foster, B.; Hart, J.C.; Proudfoot, J.; Saxon, D.H.; Woodworth, P.L.

    1982-02-01

    Current models of e+e- annihilation to baryons are reviewed and compared to the available data. Since the experimental predictions of most models are found to be very similar, an attempt is made to find differences between them which can be tested as more data become available. (author)

  2. Contribution for study on positron annihilation in tris (dipivaloilmethanates) lanthanides (III)

    International Nuclear Information System (INIS)

    Ribeiro e Silva, M.E.S.

    1988-01-01

    Some data on life time of positron and annihilation by Doppler effect in tris (dipivaloilmethanates) lanthanides (III), Ln (dpm) 3 , and Ln = Eu, Gd, Dy, Ho, Er, Tm and Yb are shown. Some results from positronium (Ps) in complexes except Eu (dpm) 3 , chemical aspects and properties of positron and positronium are evaluated. (M.J.C.) [pt

  3. Annihilation gamma ray background characterization and rejection for a positron camera

    International Nuclear Information System (INIS)

    Levin, C.S.; Tornai, M.P.; MacDonald, L.R.

    1996-01-01

    We have developed a miniature (1.2 cm 2 ) beta-ray camera prototype to assist a surgeon in locating and removing the margins of a resected tumor. When imaging positron emitting radiopharmaceuticals, annihilation gamma ray interactions in the detector can mimic those of the betas. The extent of the background contamination depends on the detector, geometry and tumor specificity of the radiopharmaceutical. We have characterized the effects that annihilation gamma rays have on positron imaging with the camera. We studied beta and gamma ray detection rates and imaging using small positron or electron sources directly exposed to the detector to simulate hot tumor remnants and a cylinder filled with 18 F to simulate annihilation background from the brain. For various ratios of phantom brain/tumor activity, a annihilation gamma rate of 1.8 cts/sec/gCi was measured in the CaF 2 (Eu) detector. We present two gamma-ray background rejection schemes that use a β-γ coincidence. Results show that the coincidence methods works with ∼99% gamma ray rejection efficiency

  4. DLTS study of annihilation of oxidation induced deep-level defects ...

    Indian Academy of Sciences (India)

    This paper describes the fabrication of MOS capacitor and DLTS study of annihilation of deeplevel defects upon thermal annealing. Ni/SiO2/-Si MOS structures fabricated on -type Si wafers were investigated for process-induced deep-level defects. The deep-level traps in Si substrates induced during the processing of ...

  5. Negative binomial distribution for multiplicity distributions in e/sup +/e/sup -/ annihilation

    International Nuclear Information System (INIS)

    Chew, C.K.; Lim, Y.K.

    1986-01-01

    The authors show that the negative binomial distribution fits excellently the available charged-particle multiplicity distributions of e/sup +/e/sup -/ annihilation into hadrons at three different energies √s = 14, 22 and 34 GeV

  6. Search for right-handed neutrinos from dark matter annihilation with gamma-rays

    Energy Technology Data Exchange (ETDEWEB)

    Campos, Miguel D.; Queiroz, Farinaldo S.; Yaguna, Carlos E. [Max-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg (Germany); Weniger, Christoph, E-mail: miguel.campos@mpi-hd.mpg.de, E-mail: farinaldo.queiroz@mpi-hd.mpg.de, E-mail: carlos.yaguna@uptc.edu.co, E-mail: c.weniger@uva.nl [GRAPPA, Institute of Physics, University of Amsterdam, Science Park 904, 1090 GL Amsterdam (Netherlands)

    2017-07-01

    Several extensions of the Standard Model contain right-handed (sterile) neutrinos in the GeV-TeV mass range. Due to their mixing with the active neutrinos, they may give rise to novel effects in cosmology, neutrino physics, and collider searches. In addition, right-handed neutrinos can also appear as final states from dark matter annihilations, with important implications for dark matter indirect detection searches. In this paper, we use current data from the Fermi Large Area Telescope (6-year observation of dwarf spheroidal galaxies) and H.E.S.S. (10-year observation of the Galactic center) to constrain the annihilation of dark matter into right-handed neutrinos. We consider right-handed neutrino with masses between 10 GeV and 1 TeV, including both two-body and three-body decays, to derive bounds on the dark matter annihilation rate, ( σ v ), as a function of the dark matter mass. Our results show, in particular, that the thermal dark matter annihilation cross section, 3× 10{sup −26} cm{sup 3} s {sup −1} , into right-handed neutrinos is excluded for dark matter masses smaller than 200 GeV.

  7. First search for dark matter annihilations in the Earth with the IceCube detector

    Energy Technology Data Exchange (ETDEWEB)

    Aartsen, M.G.; Hill, G.C.; Robertson, S.; Wallace, A.; Whelan, B.J. [University of Adelaide, Department of Physics, Adelaide (Australia); Abraham, K.; Bernhard, A.; Coenders, S.; Holzapfel, K.; Huber, M.; Jurkovic, M.; Krings, K.; Resconi, E.; Turcati, A.; Veenkamp, J. [Technische Universitaet Muenchen, Physik-Department, Garching (Germany); Ackermann, M.; Bernardini, E.; Blot, S.; Bretz, H.P.; Franckowiak, A.; Gluesenkamp, T.; Jacobi, E.; Karg, T.; Kintscher, T.; Kunwar, S.; Mohrmann, L.; Nahnhauer, R.; Satalecka, K.; Spiering, C.; Stasik, A.; Stoessl, A.; Strotjohann, N.L.; Terliuk, A.; Usner, M.; Santen, J. van; Yanez, J.P. [DESY, Zeuthen (Germany); Adams, J. [University of Canterbury, Department of Physics and Astronomy, Private Bag 4800, Christchurch (New Zealand); Aguilar, J.A.; Ansseau, I.; Heereman, D.; Meagher, K.; Meures, T.; O' Murchadha, A.; Pinat, E.; Raab, C. [Universite Libre de Bruxelles, Science Faculty CP230, Brussels (Belgium); Ahlers, M.; Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J.C.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Griffith, Z.; Halzen, F.; Hanson, K.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J.L.; Kheirandish, A.; Krueger, C.; Mancina, S.; McNally, F.; Merino, G.; Sabbatini, L.; Tobin, M.N.; Tosi, D.; Vandenbroucke, J.; Rossem, M. van; Wandkowsky, N.; Wendt, C.; Westerhoff, S.; Wille, L.; Xu, D.L. [University of Wisconsin, Department of Physics and Wisconsin IceCube Particle Astrophysics Center, Madison, WI (United States); Ahrens, M.; Bohm, C.; Dumm, J.P.; Finley, C.; Flis, S.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M. [Stockholm University, Department of Physics, Oskar Klein Centre, Stockholm (Sweden); Altmann, D.; Anton, G.; Katz, U.; Kittler, T.; Tselengidou, M. [Friedrich-Alexander-Universitaet Erlangen-Nuernberg, Centre for Astroparticle Physics, Erlangen (Germany); Andeen, K. [Marquette University, Department of Physics, Milwaukee, WI (United States); Anderson, T.; Dunkman, M.; Eller, P.; Huang, F.; Keivani, A.; Lanfranchi, J.L.; Pankova, D.V.; Quinnan, M.; Tesic, G.; Weiss, M.J. [Pennsylvania State University, Department of Physics, University Park, PA (United States); Archinger, M.; Baum, V.; Boeser, S.; Pino Rosendo, E. del; Di Lorenzo, V.; Eberhardt, B.; Ehrhardt, T.; Foesig, C.C.; Koepke, L.; Krueckl, G.; Peiffer, P.; Sandroos, J.; Steuer, A.; Wiebe, K. [University of Mainz, Institute of Physics, Mainz (Germany); Argueelles, C.; Axani, S.; Collin, G.H.; Conrad, J.M.; Jones, B.J.P.; Moulai, M. [Massachusetts Institute of Technology, Department of Physics, Cambridge, MA (United States); Auffenberg, J.; Bissok, M.; Glagla, M.; Glauch, T.; Haack, C.; Hansmann, B.; Hansmann, T.; Kemp, J.; Konietz, R.; Leuermann, M.; Leuner, J.; Penek, Oe.; Raedel, L.; Reimann, R.; Rongen, M.; Schimp, M.; Schoenen, S.; Schumacher, L.; Stahlberg, M.; Stettner, J.; Vehring, M.; Vogel, E.; Wallraff, M.; Wickmann, S.; Wiebusch, C.H. [RWTH Aachen University, III. Physikalisches Institut, Aachen (Germany); Bai, X. [South Dakota School of Mines and Technology, Physics Department, Rapid City, SD (United States); Barwick, S.W.; Yodh, G. [University of California, Department of Physics and Astronomy, Irvine, CA (United States); Bay, R.; Filimonov, K.; Price, P.B.; Woschnagg, K. [University of California, Department of Physics, Berkeley, CA (United States); Beatty, J.J. [Ohio State University, Department of Physics and Center for Cosmology and Astro-Particle Physics, Columbus, OH (United States); Ohio State University, Department of Astronomy, Columbus, OH (United States); Becker Tjus, J.; Bos, F.; Eichmann, B.; Kroll, M.; Mandelartz, M.; Schoeneberg, S.; Tenholt, F. [Ruhr-Universitaet Bochum, Fakultaet fuer Physik and Astronomie, Bochum (Germany); Becker, K.H.; Bindig, D.; Helbing, K.; Hickford, S.; Hoffmann, R.; Kopper, S.; Lauber, F.; Naumann, U.; Obertacke Pollmann, A.; Soldin, D. [University of Wuppertal, Department of Physics, Wuppertal (Germany); BenZvi, S.; Cross, R. [University of Rochester, Department of Physics and Astronomy, Rochester, NY (United States); Berley, D.; Blaufuss, E.; Cheung, E.; Felde, J.; Friedman, E.; Hellauer, R.; Hoffman, K.D.; Maunu, R.; Olivas, A.; Schmidt, T.; Song, M.; Sullivan, G.W. [University of Maryland, Department of Physics, College Park, MD (United States); Besson, D.Z. [University of Kansas, Department of Physics and Astronomy, Lawrence, KS (United States); Binder, G.; Gerhardt, L.; Klein, S.R.; Miarecki, S.; Tatar, J. [University of California, Department of Physics, Berkeley, CA (United States); Lawrence Berkeley National Laboratory, Berkeley, CA (United States); Collaboration: IceCube Collaboration; and others

    2017-02-15

    We present the results of the first IceCube search for dark matter annihilation in the center of the Earth. Weakly interacting massive particles (WIMPs), candidates for dark matter, can scatter off nuclei inside the Earth and fall below its escape velocity. Over time the captured WIMPs will be accumulated and may eventually self-annihilate. Among the annihilation products only neutrinos can escape from the center of the Earth. Large-scale neutrino telescopes, such as the cubic kilometer IceCube Neutrino Observatory located at the South Pole, can be used to search for such neutrino fluxes. Data from 327 days of detector livetime during 2011/2012 were analyzed. No excess beyond the expected background from atmospheric neutrinos was detected. The derived upper limits on the annihilation rate of WIMPs in the Earth and the resulting muon flux are an order of magnitude stronger than the limits of the last analysis performed with data from IceCube's predecessor AMANDA. The limits can be translated in terms of a spin-independent WIMP-nucleon cross section. For a WIMP mass of 50 GeV this analysis results in the most restrictive limits achieved with IceCube data. (orig.)

  8. A study on lead myristate (LM) soap film crystal by positron annihilation life spectroscopy

    International Nuclear Information System (INIS)

    Shi Zikang; Yu xianchun

    1992-01-01

    The quality of the LM soap film crystal is determined by means of the positron annihilation life spectroscopy. It is found that the technology to be used to make soap film will influence the film quality and the film quality can be improved by a reasonable heat treatment

  9. Dark matter annihilations into two light fermions and one gauge boson. General analysis and antiproton constraints

    International Nuclear Information System (INIS)

    Garny, Mathias; Ibarra, Alejandro; Vogl, Stefan

    2011-12-01

    We study in this paper the scenario where the dark matter is constituted by Majo- rana particles which couple to a light Standard Model fermion and an extra scalar via a Yukawa coupling. In this scenario, the annihilation rate into the light fermions with the mediation of the scalar particle is strongly suppressed by the mass of the fermion. Nevertheless, the helicity suppression is lifted by the associated emission of a gauge boson, yielding annihilation rates which could be large enough to allow the indirect detection of the dark matter particles. We perform a general analysis of this scenario, calculating the annihilation cross section of the processes χχ → f anti fV when the dark matter particle is a SU(2) L singlet or doublet, f is a lepton or a quark, and V is a photon, a weak gauge boson or a gluon. We point out that the annihilation rate is particularly enhanced when the dark matter particle is degenerate in mass to the intermediate scalar particle, which is a scenario barely constrained by collider searches of exotic charged or colored particles. Lastly, we derive upper limits on the relevant cross sections from the non-observation of an excess in the cosmic antiproton-to-proton ratio measured by PAMELA. (orig.)

  10. Annihilation vs. decay: constraining dark matter properties from a gamma-ray detection

    International Nuclear Information System (INIS)

    Palomares-Ruiz, Sergio; Siegal-Gaskins, Jennifer M.

    2010-01-01

    Most proposed dark matter candidates are stable and are produced thermally in the early Universe. However, there is also the possibility of unstable (but long-lived) dark matter, produced thermally or otherwise. We propose a strategy to distinguish between dark matter annihilation and/or decay in the case that a clear signal is detected in gamma-ray observations of Milky Way dwarf spheroidal galaxies with gamma-ray experiments. The sole measurement of the energy spectrum of an indirect signal would render the discrimination between these cases impossible. We show that by examining the dependence of the intensity and energy spectrum on the angular distribution of the emission, the origin could be identified as decay, annihilation, or both. In addition, once the type of signal is established, we show how these measurements could help to extract information about the dark matter properties, including mass, annihilation cross section, lifetime, dominant annihilation and decay channels, and the presence of substructure. Although an application of the approach presented here would likely be feasible with current experiments only for very optimistic dark matter scenarios, the improved sensitivity of upcoming experiments could enable this technique to be used to study a wider range of dark matter models

  11. Annihilation vs. decay: constraining dark matter properties from a gamma-ray detection

    Energy Technology Data Exchange (ETDEWEB)

    Palomares-Ruiz, Sergio [Centro de Física Teórica de Partículas, Instituto Superior Técnico, Av. Rovisco Pais 1, 1049-001 Lisboa (Portugal); Siegal-Gaskins, Jennifer M., E-mail: sergio.palomares.ruiz@ist.utl.pt, E-mail: jsg@mps.ohio-state.edu [Center for Cosmology and AstroParticle Physics, The Ohio State University, 191 W. Woodruff Ave., Columbus OH 43210 (United States)

    2010-07-01

    Most proposed dark matter candidates are stable and are produced thermally in the early Universe. However, there is also the possibility of unstable (but long-lived) dark matter, produced thermally or otherwise. We propose a strategy to distinguish between dark matter annihilation and/or decay in the case that a clear signal is detected in gamma-ray observations of Milky Way dwarf spheroidal galaxies with gamma-ray experiments. The sole measurement of the energy spectrum of an indirect signal would render the discrimination between these cases impossible. We show that by examining the dependence of the intensity and energy spectrum on the angular distribution of the emission, the origin could be identified as decay, annihilation, or both. In addition, once the type of signal is established, we show how these measurements could help to extract information about the dark matter properties, including mass, annihilation cross section, lifetime, dominant annihilation and decay channels, and the presence of substructure. Although an application of the approach presented here would likely be feasible with current experiments only for very optimistic dark matter scenarios, the improved sensitivity of upcoming experiments could enable this technique to be used to study a wider range of dark matter models.

  12. Total cross section for hadron production by electron-positron annihilation at ADONE

    International Nuclear Information System (INIS)

    Ambrosio, M.; Paternoster, G.; Tortora, L.; Troya, U.; Bemporad, C.; Brosco, G.; Calvetti, M.; Costantini, F.; Giannini, G.R.; Lariccia, P.; Pisa Univ.

    1980-01-01

    The total cross section for electron-positron annihilation into three or more hadrons has been measured for centre of mass energies between 1.4 and 2.0 GeV. The data were obtained at ADONE by the B anti B experiment. (orig.)

  13. Forty-five years of e+e- annihilation physics: 1956 to 2001

    International Nuclear Information System (INIS)

    Richter, B.

    1985-04-01

    The history of e + e - physics in the 1950's and 1960's is reviewed, followed by some highlights of the spectacular discoveries in e + e - annihilation made during the 1970's. The consolidation of knowledge during the last few years is summarized. Some predictions are made for the field of e + e - physics for the next decade and beyond

  14. Heating of galactic gas by dark matter annihilation in ultracompact minihalos

    Energy Technology Data Exchange (ETDEWEB)

    Clark, Hamish A.; Iwanus, Nikolas; Lewis, Geraint F. [Sydney Institute for Astronomy, School of Physics A28, The University of Sydney, NSW 2006 (Australia); Elahi, Pascal J. [International Centre for Radio Astronomy Research, University of Western Australia, 35 Stirling Highway, Crawley, WA 6009 (Australia); Scott, Pat, E-mail: hamish.clark@sydney.edu.au, E-mail: nikolas.iwanus@sydney.edu.au, E-mail: pascal.elahi@uwa.edu.au, E-mail: geraint.lewis@sydney.edu.au, E-mail: p.scott@imperial.ac.uk [Department of Physics, Imperial College London, Blackett Laboratory, Prince Consort Road, London SW7 2AZ (United Kingdom)

    2017-05-01

    The existence of substructure in halos of annihilating dark matter would be expected to substantially boost the rate at which annihilation occurs. Ultracompact minihalos of dark matter (UCMHs) are one of the more extreme examples of this. The boosted annihilation can inject significant amounts of energy into the gas of a galaxy over its lifetime. Here we determine the impact of the boost factor from UCMH substructure on the heating of galactic gas in a Milky Way-type galaxy, by means of N-body simulation. If 1% of the dark matter exists as UCMHs, the corresponding boost factor can be of order 10{sup 5}. For reasonable values of the relevant parameters (annihilation cross section 3×10{sup −26} cm{sup 3} s{sup −1}, dark matter mass 100 GeV, 10% heating efficiency), we show that the presence of UCMHs at the 0.1% level would inject enough energy to eject significant amounts of gas from the halo, potentially preventing star formation within ∼1 kpc of the halo centre.

  15. Positron annihilation study on Y-Ba-Cu-O high Tc superconductors

    International Nuclear Information System (INIS)

    Balogh, A.G.; Liszkay, L.; Molnar, B.; Puff, W.

    1987-08-01

    First positron annihilation measurements are reported on high T c superconductor YBa 2 Cu 3 O 7-x . The lifetime and Doppler broadening spectra show a slight but significant change about 240K suggesting a deviation from the normal structure far above 90K where the resistance falls to zero. (author)

  16. Quantum efficiency harmonic analysis of exciton annihilation in organic light emitting diodes

    Energy Technology Data Exchange (ETDEWEB)

    Price, J. S.; Giebink, N. C., E-mail: ncg2@psu.edu [Department of Electrical Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802 (United States)

    2015-06-29

    Various exciton annihilation processes are known to impact the efficiency roll-off of organic light emitting diodes (OLEDs); however, isolating and quantifying their contribution in the presence of other factors such as changing charge balance continue to be a challenge for routine device characterization. Here, we analyze OLED electroluminescence resulting from a sinusoidal dither superimposed on the device bias and show that nonlinearity between recombination current and light output arising from annihilation mixes the quantum efficiency measured at different dither harmonics in a manner that depends uniquely on the type and magnitude of the annihilation process. We derive a series of analytical relations involving the DC and first harmonic external quantum efficiency that enable annihilation rates to be quantified through linear regression independent of changing charge balance and evaluate them for prototypical fluorescent and phosphorescent OLEDs based on the emitters 4-(dicyanomethylene)-2-methyl-6-(4-dimethylaminostyryl)-4H-pyran and platinum octaethylporphyrin, respectively. We go on to show that, in most cases, it is sufficient to calculate the needed quantum efficiency harmonics directly from derivatives of the DC light versus current curve, thus enabling this analysis to be conducted solely from standard light-current-voltage measurement data.

  17. Some aspects of free volume studies in molecular substances using positron annihilation experiments

    International Nuclear Information System (INIS)

    Shantarovich, V.P.; Gustov, V.W.; Kevdina, I.B.; Suzuki, T.; Djourelov, N.; Shimazu, A.

    2005-01-01

    Positron annihilation lifetime spectroscopy is accepted now as a method for the studies of elementary free volumes (free volume holes) in solids, in polymers in particular. The aim of this paper is to discuss some problems, the difficulties on the way of this application and to illustrate them by several examples obtained by the authors. (author)

  18. Hyperfine splitting in positronium to O(α7me). One-photon annihilation contribution

    International Nuclear Information System (INIS)

    Baker, M.; Penin, A.A.; Karlsruher Institut fuer Technologie; Piclum, J.; RWTH Aachen; Steinhauser, M.

    2014-02-01

    We present the complete result for the O(α 7 m e ) one-photon annihilation contribution to the hyperfine splitting of the ground state energy levels in positronium. Numerically it increases the prediction of quantum electrodynamics by 217±1 kHz.

  19. A Monte Carlo model to produce baryons in e+e- annihilation

    International Nuclear Information System (INIS)

    Meyer, T.

    1981-08-01

    A simple model is described extending the Field-Feynman model to baryon production in quark fragmentation. The model predicts baryon baryon correlations within jets and in opposite jets produced in electron-positron annihilation. Existing data is well described by the model. (orig.)

  20. The need for expanded exploration of matter-antimatter annihilation for propulsion application

    Science.gov (United States)

    Massier, P. F.

    1982-01-01

    The use of matter-antimatter annihilation as a propulsion application for interstellar travel is discussed. The physical basis for the superior energy release in such a system is summarized, and the problems associated with antimatter production, collection and storage are assessed. Advances in devising a workable propulsion system are reported, and the parameters of an antimatter propulsion system are described.

  1. Toward a minimum branching fraction for dark matter annihilation into electromagnetic final states

    International Nuclear Information System (INIS)

    Dent, James B.; Scherrer, Robert J.; Weiler, Thomas J.

    2008-01-01

    Observational limits on the high-energy neutrino background have been used to place general constraints on dark matter that annihilates only into standard model particles. Dark matter particles that annihilate into neutrinos will also inevitably branch into electromagnetic final states through higher-order tree and loop diagrams that give rise to charged leptons, and these charged particles can transfer their energy into photons via synchrotron radiation or inverse Compton scattering. In the context of effective field theory, we calculate the loop-induced branching ratio to charged leptons and show that it is generally quite large, typically > or approx. 1%, when the scale of the dark matter mass exceeds the electroweak scale, M W . For a branching fraction >or approx. 3%, the synchrotron radiation bounds on dark matter annihilation are currently stronger than the corresponding neutrino bounds in the interesting mass range from 100 GeV to 1 TeV. For dark matter masses below M W , our work provides a plausible framework for the construction of a model for 'neutrinos-only' dark matter annihilations.

  2. DLTS study of annihilation of oxidation induced deep-level defects ...

    Indian Academy of Sciences (India)

    Administrator

    †Sensors and Nanotechnology Group, Central Electronics Engineering Research Institute, Pilani 333 031, India. ††Department of Physics, Bangalore University, Bangalore 560 056, India. MS received 31 May 2010. Abstract. This paper describes the fabrication of MOS capacitor and DLTS study of annihilation of deep-.

  3. Photochemically deoxygenating solvents for triplet-triplet annihilation photon upconversion operating in air.

    Science.gov (United States)

    Wan, Shigang; Lin, Jinxiong; Su, Huimin; Dai, Junfeng; Lu, Wei

    2018-04-03

    Sulfoxides and cyclic ureas are photochemically deoxygenating solvents in which the oxidative stress could be released and efficient triplet-triplet annihilation photon upconversion (TTA-UC) can operate in air. Such solvents can be practically screened out by harnessing the property of photo-activated phosphorescence.

  4. A Positron Annihilation Study of Copper Containing a High Concentration of Krypton

    DEFF Research Database (Denmark)

    Eldrup, Morten Mostgaard; Evans, John H.

    1982-01-01

    Bulk Cu samples containing up to 4 at.% Kr have been produced by the Harwell combined ion implantation and sputtering method at temperatures near ambient, and then examined by the positron annihilation technique. Both angular correlation and lifetime measurements were made and, in addition...

  5. Review of Heavy Lepton Production in e{sup +}e{sup -} Annihilation

    Science.gov (United States)

    Perl, M. L.

    1977-10-01

    The existing data on e{sup +-}..mu..{sup -+}, e{sup +-}x{sup -+}, ..mu..{sup +-}x{sup -+}, and related events produced in e{sup +}e{sup -} annihilation are reviewed. All data are consistent with the existence of a new charged lepton, tau{sup +-}, of mass 1.9 +- .1 GeV/c{sup 2}.

  6. Doing the "Second Shift": Gendered Labour and the Symbolic Annihilation of Teacher Educators' Work

    Science.gov (United States)

    Spencer, Ingrid

    2013-01-01

    Reflecting on the experience of being a participant in the Work of Teacher Education (WoTE) research, and drawing on conceptualisations of teacher education as "domestic labour," I argue that teacher educators' closeness to classroom practice acts as a determining factor in their symbolic annihilation, a concept usually applied to study…

  7. A positron annihilation spectroscopic investigation of europium-doped cerium oxide nanoparticles.

    Science.gov (United States)

    Thorat, Atul V; Ghoshal, Tandra; Holmes, Justin D; Nambissan, P M G; Morris, Michael A

    2014-01-07

    Doping in ceria (CeO2) nanoparticles with europium (Eu) of varying concentrations (0, 0.1, 0.5, …, 50 atom%) is studied using complementary experimental techniques and novel observations were made during the investigation. The immediate observable effect was a distinct reduction in particle sizes with increasing Eu concentration attributed to the relaxation of strain introduced due to the replacement of Ce(4+) ions by Eu(3+) ions of larger radius. However, this general trend was reversed in the doping concentration range of 0.1-1 atom% due to the reduction of Ce(4+) to Ce(3+) and the formation of anion vacancies. Quantum confinement effects became evident with the increase of band gap energy when the particle sizes reduced below 7-8 nm. Positron annihilation studies indicated the presence of vacancy type defects in the form of vacancy clusters within the nanoparticles. Some positron annihilation was also seen on the surface of crystallites as a result of diffusion of thermalized positrons before annihilation. Coincidence Doppler broadening measurements indicated the annihilation of positrons with electrons of different species of atoms and the characteristic S-W plot showed a kink-like feature at the particle sizes where quantum confinement effects began.

  8. Pick-off annihilation of positronium in matter using full correlation single particle potentials: solid He.

    Science.gov (United States)

    Zubiaga, A; Tuomisto, F; Puska, M J

    2015-01-29

    We investigate the modeling of positronium (Ps) states and their pick-off annihilation trapped at open volumes pockets in condensed molecular matter. Our starting point is the interacting many-body system of Ps and a He atom because it is the smallest entity that can mimic the energy gap between the highest occupied and lowest unoccupied molecular orbitals of molecules, and yet the many-body structure of the HePs system can be calculated accurately enough. The exact-diagonalization solution of the HePs system enables us to construct a pairwise full-correlation single-particle potential for the Ps-He interaction, and the total potential in solids is obtained as a superposition of the pairwise potentials. We study in detail Ps states and their pick-off annihilation rates in voids inside solid He and analyze experimental results for Ps-induced voids in liquid He obtaining the radii of the voids. More importantly, we generalize our conclusions by testing the validity of the Tao-Eldrup model, widely used to analyze ortho-Ps annihilation measurements for voids in molecular matter, against our theoretical results for the solid He. Moreover, we discuss the influence of the partial charges of polar molecules and the strength of the van der Waals interaction on the pick-off annihilation rate.

  9. Reflection, transmutation, annihilation, and resonance in two-component kink collisions

    Science.gov (United States)

    Alonso-Izquierdo, A.

    2018-02-01

    In this paper, the study of collisions between kinks arising in the family of MSTB models is addressed. Phenomena such as elastic kink reflection, mutual annihilation, kink-antikink transmutation and inelastic reflection are found and depend on the impact velocity.

  10. Positron annihilation lifetime studies of SrTiO.sub.3./sub. crystal and ceramic materials

    Czech Academy of Sciences Publication Activity Database

    Keeble, D.J.; McGuire, R.; Singh, S.; Su, B.; Button, T.W.; Petzelt, Jan

    2005-01-01

    Roč. 128, - (2005), s. 111-114 ISSN 1155-4339 Institutional research plan: CEZ:AV0Z10100520 Keywords : positron annihilation * SrTiO 3 crystal * spectroscopy Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 0.389, year: 2005

  11. Direct Detection Phenomenology in Models Where the Products of Dark Matter Annihilation Interact with Nuclei.

    Science.gov (United States)

    Cherry, John F; Frandsen, Mads T; Shoemaker, Ian M

    2015-06-12

    We investigate the direct detection phenomenology of a class of dark matter (DM) models in which DM does not directly interact with nuclei, but rather, the products of its annihilation do. When these annihilation products are very light compared to the DM mass, the scattering in direct detection experiments is controlled by relativistic kinematics. This results in a distinctive recoil spectrum, a nonstandard and/or even absent annual modulation, and the ability to probe DM masses as low as a ∼10  MeV. We use current LUX data to show that experimental sensitivity to thermal relic annihilation cross sections has already been reached in a class of models. Moreover, the compatibility of dark matter direct detection experiments can be compared directly in Emin space without making assumptions about DM astrophysics, mass, or scattering form factors. Lastly, when DM has direct couplings to nuclei, the limit from annihilation to relativistic particles in the Sun can be stronger than that of conventional nonrelativistic direct detection by more than 3 orders of magnitude for masses in a 2-7 GeV window.

  12. Interpretation of the gamma-ray excess and AMS-02 antiprotons: Velocity dependent dark matter annihilations

    Science.gov (United States)

    Jia, Lian-Bao

    2017-09-01

    The two messenger results of the GeV gamma-ray excess at the Galactic center and a probable antiproton excess in the recent AMS-02 observation suggest that these two anomalies may be owing to the same origin—the dark matter (DM) annihilation into b b ¯, while these results seem in tension with the dwarf spheroidal galaxy observations. To give a compatible explanation about it, we consider the pseudoscalar DM particles Sd+Sd- annihilating via Sd+Sd-→Sd0Sd0, with the process mediated by a new scalar ϕ and Sd0 quickly decaying into b b ¯. For the particles Sd+, Sd-, and Sd0 in a triplet with degenerate masses, the annihilation cross section of DM today is linearly dependent on the relative velocity vr, and thus constraints from the dwarf spheroidal galaxies are relaxed. The parameter spaces are derived with corresponding constraints. Though traces from the new sector seem challenging to be disclosed at the collider and in DM direct detections, the indirect search of the gamma-ray line from the Sd0's decay has the potential to shed light on DM annihilations, with the energy of the gamma-ray line ˜mSd0/2 , i.e. about 50-75 GeV.

  13. The study of synthetic food dyes by positron annihilation lifetime spectroscopy.

    Science.gov (United States)

    Pivtsaev, A. A.; Razov, V. I.

    2015-06-01

    By method of positron annihilation lifetime spectroscopy (PALS), substances are food dyes were studied: E-102 (Tartrazine), E-124 (Ponso 4R), E 132 (Indigo carmine), E-133 (Brilliant Blue), E-151 (Black Shiny). They are examined for the presence of carcinogenic properties. The difference between dyes having explicit carcinogenic properties and mutagenic properties (non-explicit carcinogens) is established.

  14. The study of synthetic food dyes by positron annihilation lifetime spectroscopy

    International Nuclear Information System (INIS)

    Pivtsaev, A A; Razov, V I

    2015-01-01

    By method of positron annihilation lifetime spectroscopy (PALS), substances are food dyes were studied: E-102 (Tartrazine), E-124 (Ponso 4R), E 132 (Indigo carmine), E-133 (Brilliant Blue), E-151 (Black Shiny). They are examined for the presence of carcinogenic properties. The difference between dyes having explicit carcinogenic properties and mutagenic properties (non-explicit carcinogens) is established. (paper)

  15. Multi-messenger constraints and pressure from dark matter annihilation into e--e+ pairs

    International Nuclear Information System (INIS)

    Wechakama, Maneenate

    2013-01-01

    Despite striking evidence for the existence of dark matter from astrophysical observations, dark matter has still escaped any direct or indirect detection until today. Therefore a proof for its existence and the revelation of its nature belongs to one of the most intriguing challenges of nowadays cosmology and particle physics. The present work tries to investigate the nature of dark matter through indirect signatures from dark matter annihilation into electron-positron pairs in two different ways, pressure from dark matter annihilation and multi-messenger constraints on the dark matter annihilation cross-section. We focus on dark matter annihilation into electron-positron pairs and adopt a model-independent approach, where all the electrons and positrons are injected with the same initial energy E 0 ∝m dm c 2 . The propagation of these particles is determined by solving the diffusion-loss equation, considering inverse Compton scattering, synchrotron radiation, Coulomb collisions, bremsstrahlung, and ionization. The first part of this work, focusing on pressure from dark matter annihilation, demonstrates that dark matter annihilation into electron-positron pairs may affect the observed rotation curve by a significant amount. The injection rate of this calculation is constrained by INTEGRAL, Fermi, and H.E.S.S. data. The pressure of the relativistic electron-positron gas is computed from the energy spectrum predicted by the diffusion-loss equation. For values of the gas density and magnetic field that are representative of the Milky Way, it is estimated that the pressure gradients are strong enough to balance gravity in the central parts if E 0 0 . By comparing the predicted rotation curves with observations of dwarf and low surface brightness galaxies, we show that the pressure from dark matter annihilation may improve the agreement between theory and observations in some cases, but it also imposes severe constraints on the model parameters (most notably, the

  16. Prospects for discovering a neutrino line induced by dark matter annihilation

    Science.gov (United States)

    El Aisati, Chaimae; Garcia-Cely, Camilo; Hambye, Thomas; Vanderheyden, Laurent

    2017-10-01

    In the near future, neutrino telescopes are expected to improve their sensitivity to the flux of monochromatic neutrinos produced by dark matter (DM) in our galaxy. This is illustrated by a new limit on the corresponding cross section that we derive from public IceCube data. In this context, we study which DM models could produce an observable flux of monochromatic neutrinos from DM annihilations. To this end, we proceed in two steps. First, within a set of simple and minimal assumptions concerning the properties of the DM particle, we determine the models that could give rise to a significant annihilation into monochromatic neutrinos at the freeze-out epoch. The list of models turns out to be very limited as a result of various constraints, in particular direct detection and neutrino masses at loop level. Given the fact that, even if largely improved, the sensitivities will be far from reaching the thermal annihilation cross section soon, a signal could only be observed if the annihilation into neutrinos today is boosted with respect to the freeze-out epoch. This is why, in a second step, we analyze the possibility of having such a large enhancement from the Sommerfeld effect. For each scenario, we also compute the cross sections into other annihilation products and confront our results with experimental constraints. We find that, within our simple and minimal assumptions, the expectation to observe monochromatic neutrinos is only possible in very specific scenarios. Some will be confirmed or excluded in the near future because they predict signals slightly below the current experimental sensitivities. We also discuss how these prospects change by relaxing our assumptions as well as by considering other types of sharp spectral features. For the latter, we consider boxed-shaped and bremsstrahlung spectra and provide the corresponding limits from IceCube data.

  17. Limits on a muon flux from neutralino annihilations in the sun with the IceCube 22-string detector.

    Science.gov (United States)

    Abbasi, R; Abdou, Y; Ackermann, M; Adams, J; Ahlers, M; Andeen, K; Auffenberg, J; Bai, X; Baker, M; Barwick, S W; Bay, R; Bazo Alba, J L; Beattie, K; Beatty, J J; Bechet, S; Becker, J K; Becker, K-H; Benabderrahmane, M L; Berdermann, J; Berghaus, P; Berley, D; Bernardini, E; Bertrand, D; Besson, D Z; Bissok, M; Blaufuss, E; Boersma, D J; Bohm, C; Bolmont, J; Böser, S; Botner, O; Bradley, L; Braun, J; Breder, D; Burgess, T; Castermans, T; Chirkin, D; Christy, B; Clem, J; Cohen, S; Cowen, D F; D'Agostino, M V; Danninger, M; Day, C T; De Clercq, C; Demirörs, L; Depaepe, O; Descamps, F; Desiati, P; de Vries-Uiterweerd, G; Deyoung, T; Diaz-Velez, J C; Dreyer, J; Dumm, J P; Duvoort, M R; Edwards, W R; Ehrlich, R; Eisch, J; Ellsworth, R W; Engdegård, O; Euler, S; Evenson, P A; Fadiran, O; Fazely, A R; Feusels, T; Filimonov, K; Finley, C; Foerster, M M; Fox, B D; Franckowiak, A; Franke, R; Gaisser, T K; Gallagher, J; Ganugapati, R; Gerhardt, L; Gladstone, L; Goldschmidt, A; Goodman, J A; Gozzini, R; Grant, D; Griesel, T; Gross, A; Grullon, S; Gunasingha, R M; Gurtner, M; Ha, C; Hallgren, A; Halzen, F; Han, K; Hanson, K; Hasegawa, Y; Heise, J; Helbing, K; Herquet, P; Hickford, S; Hill, G C; Hoffman, K D; Hoshina, K; Hubert, D; Huelsnitz, W; Hülss, J-P; Hulth, P O; Hultqvist, K; Hussain, S; Imlay, R L; Inaba, M; Ishihara, A; Jacobsen, J; Japaridze, G S; Johansson, H; Joseph, J M; Kampert, K-H; Kappes, A; Karg, T; Karle, A; Kelley, J L; Kenny, P; Kiryluk, J; Kislat, F; Klein, S R; Klepser, S; Knops, S; Kohnen, G; Kolanoski, H; Köpke, L; Kowalski, M; Kowarik, T; Krasberg, M; Kuehn, K; Kuwabara, T; Labare, M; Lafebre, S; Laihem, K; Landsman, H; Lauer, R; Leich, H; Lennarz, D; Lucke, A; Lundberg, J; Lünemann, J; Madsen, J; Majumdar, P; Maruyama, R; Mase, K; Matis, H S; McParland, C P; Meagher, K; Merck, M; Mészáros, P; Middell, E; Milke, N; Miyamoto, H; Mohr, A; Montaruli, T; Morse, R; Movit, S M; Münich, K; Nahnhauer, R; Nam, J W; Niessen, P; Nygren, D R; Odrowski, S; Olivas, A; Olivo, M; Ono, M; Panknin, S; Patton, S; Pérez de Los Heros, C; Petrovic, J; Piegsa, A; Pieloth, D; Pohl, A C; Porrata, R; Potthoff, N; Price, P B; Prikockis, M; Przybylski, G T; Rawlins, K; Redl, P; Resconi, E; Rhode, W; Ribordy, M; Rizzo, A; Rodrigues, J P; Roth, P; Rothmaier, F; Rott, C; Roucelle, C; Rutledge, D; Ryckbosch, D; Sander, H-G; Sarkar, S; Satalecka, K; Schlenstedt, S; Schmidt, T; Schneider, D; Schukraft, A; Schulz, O; Schunck, M; Seckel, D; Semburg, B; Seo, S H; Sestayo, Y; Seunarine, S; Silvestri, A; Slipak, A; Spiczak, G M; Spiering, C; Stamatikos, M; Stanev, T; Stephens, G; Stezelberger, T; Stokstad, R G; Stoufer, M C; Stoyanov, S; Strahler, E A; Straszheim, T; Sulanke, K-H; Sullivan, G W; Swillens, Q; Taboada, I; Tarasova, O; Tepe, A; Ter-Antonyan, S; Terranova, C; Tilav, S; Tluczykont, M; Toale, P A; Tosi, D; Turcan, D; van Eijndhoven, N; Vandenbroucke, J; Van Overloop, A; Voigt, B; Walck, C; Waldenmaier, T; Walter, M; Wendt, C; Westerhoff, S; Whitehorn, N; Wiebusch, C H; Wiedemann, A; Wikström, G; Williams, D R; Wischnewski, R; Wissing, H; Woschnagg, K; Xu, X W; Yodh, G; Yoshida, S

    2009-05-22

    A search for muon neutrinos from neutralino annihilations in the Sun has been performed with the IceCube 22-string neutrino detector using data collected in 104.3 days of live time in 2007. No excess over the expected atmospheric background has been observed. Upper limits have been obtained on the annihilation rate of captured neutralinos in the Sun and converted to limits on the weakly interacting massive particle (WIMP) proton cross sections for WIMP masses in the range 250-5000 GeV. These results are the most stringent limits to date on neutralino annihilation in the Sun.

  18. Impact of semi-annihilations on dark matter phenomenology - an example of ZN symmetric scalar dark matter

    International Nuclear Information System (INIS)

    Belanger, G.; Kannike, K.; Pukhov, A.; Raidal, M.

    2012-01-01

    We study the impact of semi-annihilations χχ ↔ χX; where χ is dark matter and X is any standard model particle, on dark matter phenomenology. We formulate scalar dark matter models with minimal field content that predict non-trivial dark matter phenomenology for different discrete Abelian symmetries Z N , N > 2, and contain semi-annihilation processes. We implement such an example model in micrOMEGAs and show that semi-annihilations modify the phenomenology of this type of models. (authors)

  19. Title: Elucidation of Environmental Fate of Artificial Sweeteners (Aspartame, Acesulfame K and Saccharin) by Determining Bimolecular Rate Constants with Hydroxyl Radical at Various pH and Temperature Conditions and Possible Reaction By-Products

    Science.gov (United States)

    Teraji, T.; Arakaki, T.; Suzuka, T.

    2012-12-01

    Use of artificial sweeteners in beverages and food has been rapidly increasing because of their non-calorie nature. In Japan, aspartame, acesulfame K and sucralose are among the most widely used artificial sweeteners. Because the artificial sweeteners are not metabolized in human bodies, they are directly excreted into the environment without chemical transformations. We initiated a study to better understand the fate of artificial sweeteners in the marine environment. The hydroxyl radical (OH), the most potent reactive oxygen species, reacts with various compounds and determines the environmental oxidation capacity and the life-time of many compounds. The steady-state OH concentration and the reaction rate constants between the compound and OH are used to estimate the life-time of the compound. In this study, we determine the bimolecular rate constants between aspartame, acefulfame K and saccharin and OH at various pH and temperature conditions using a competition kinetics technique. We use hydrogen peroxide as a photochemical source of OH. Bimolecular rate constant we obtained so far for aspartame was (2.6±1.2)×109 M-1 s-1 at pH = 3.0 and (4.9±2.3)×109 M-1 s-1 at pH = 5.5. Little effect was seen by changing the temperatures between 15 and 40 oC. Activation energy (Ea) was calculated to be -1.0 kJ mol-1 at pH = 3.0, +8.5 kJ mol-1 at pH = 5.5, which could be regarded as zero. We will report bimolecular rate constants at different pHs and temperatures for acesulfame K and saccharin, as well. Possible reaction by-products for aspartame will be also reported. We will further discuss the fate of aspartame in the coastal environment.

  20. Probing sub-nano level molecular packing and correlated positron annihilation characteristics of ionic cross-linked chitosan membranes using positron annihilation spectroscopy.

    Science.gov (United States)

    Xia, Rui; Cao, Xingzhong; Gao, Meizhen; Zhang, Peng; Zeng, Minfeng; Wang, Baoyi; Wei, Long

    2017-02-01

    Chitosan, CS, cross-linked with bivalent palladium has shown enhanced mechanical and thermal properties depending on the transformation of the structure at a microscopic scale. In the present study, CS directly cross-linked by palladium cation membranes (CS-cr-PM) was prepared through a solution-casting method. Mobility of chitosan chains were greatly reduced after crosslinking, making a great reduction in the swelling ratio studied by a water-swelling degree measurement, which led to an improvement in molecular chain rigidity. In order to investigate the chain packing at the molecular level in the ionic cross-linked CS system, the structure of chemically-crosslinked CS is investigated by means of the combined use of wide angle X-ray diffraction (WAXD) and infrared measurements, and a combination of positron annihilation lifetime spectroscopy (PALS) and simultaneous coincidence Doppler broadening (CDB) spectroscopy offers coherent information on both the free-volume related sub-nano level molecular packing and the chemical surrounding of free volume nanoholes in CS-cr-PM as a function of palladium salt loading. The variations in the free volume size and size distribution have been determined through the ortho-positronium (o-Ps) lifetime and its lifetime distribution. The studies showed that a strong interaction between CS molecules and palladium cations results in the change in crystallinity in formed CS-cr-PM leading to variational chain packing density. Meanwhile, significant inhibition effects on positronium formation due to doping are observed, which could be interpreted in terms of the existence of chloride ions. Applications of positron annihilation spectroscopy to study the microstructure and correlated positron annihilation characteristics of an ionic cross-linked CS system are systematically discussed.

  1. Bimolecular reaction of CH3 + CO in solid p-H2: infrared absorption of acetyl radical (CH3CO) and CH3-CO complex.

    Science.gov (United States)

    Das, Prasanta; Lee, Yuan-Pern

    2014-06-28

    We have recorded infrared spectra of acetyl radical (CH3CO) and CH3-CO complex in solid para-hydrogen (p-H2). Upon irradiation at 248 nm of CH3C(O)Cl/p-H2 matrices, CH3CO was identified as the major product; characteristic intense IR absorption features at 2990.3 (ν9), 2989.1 (ν1), 2915.6 (ν2), 1880.5 (ν3), 1419.9 (ν10), 1323.2 (ν5), 836.6 (ν7), and 468.1 (ν8) cm(-1) were observed. When CD3C(O)Cl was used, lines of CD3CO at 2246.2 (ν9), 2244.0 (ν1), 1866.1 (ν3), 1046.7 (ν5), 1029.7 (ν4), 1027.5 (ν10), 889.1 (ν6), and 723.8 (ν7) cm(-1) appeared. Previous studies characterized only three vibrational modes of CH3CO and one mode of CD3CO in solid Ar. In contrast, upon photolysis of a CH3I/CO/p-H2 matrix with light at 248 nm and subsequent annealing at 5.1 K before re-cooling to 3.2 K, the CH3-CO complex was observed with characteristic IR features at 3165.7, 3164.5, 2150.1, 1397.6, 1396.4, and 613.0 cm(-1). The assignments are based on photolytic behavior, observed deuterium isotopic shifts, and a comparison of observed vibrational wavenumbers and relative IR intensities with those predicted with quantum-chemical calculations. This work clearly indicates that CH3CO can be readily produced from photolysis of CH3C(O)Cl because of the diminished cage effect in solid p-H2 but not from the reaction of CH3 + CO because of the reaction barrier. Even though CH3 has nascent kinetic energy greater than 87 kJ mol(-1) and internal energy ∼42 kJ mol(-1) upon photodissociation of CH3I at 248 nm, its energy was rapidly quenched so that it was unable to overcome the barrier height of ∼27 kJ mol(-1) for the formation of CH3CO from the CH3 + CO reaction; a barrierless channel for formation of a CH3-CO complex was observed instead. This rapid quenching poses a limitation in production of free radicals via bimolecular reactions in p-H2.

  2. Detection of Heteromers Formed by Cannabinoid CB1, Dopamine D2, and Adenosine A2A G-Protein-Coupled Receptors by Combining Bimolecular Fluorescence Complementation and Bioluminescence Energy Transfer

    Directory of Open Access Journals (Sweden)

    Gemma Navarro

    2008-01-01

    Full Text Available Functional interactions in signaling occur between dopamine D2 (D2R and cannabinoid CB1 (CB1R receptors, between CB1R and adenosine A2A (A2AR receptors, and between D2R and A2AR. Furthermore, direct molecular interactions have been reported for the pairs CB1R-D2R, A2AR-D2R, and CB1R-A2AR. Here a combination of bimolecular fluorescence complementation and bioluminescence energy transfer techniques was used to identify the occurrence of D2R-CB1R-A2AR hetero-oligomers in living cells.

  3. Efficient Green's Function Reaction Dynamics (GFRD) simulations for diffusion-limited, reversible reactions

    Science.gov (United States)

    Bashardanesh, Zahedeh; Lötstedt, Per

    2018-03-01

    In diffusion controlled reversible bimolecular reactions in three dimensions, a dissociation step is typically followed by multiple, rapid re-association steps slowing down the simulations of such systems. In order to improve the efficiency, we first derive an exact Green's function describing the rate at which an isolated pair of particles undergoing reversible bimolecular reactions and unimolecular decay separates beyond an arbitrarily chosen distance. Then the Green's function is used in an algorithm for particle-based stochastic reaction-diffusion simulations for prediction of the dynamics of biochemical networks. The accuracy and efficiency of the algorithm are evaluated using a reversible reaction and a push-pull chemical network. The computational work is independent of the rates of the re-associations.

  4. Investigation of the crystal lattice defects by means of the positrons annihilations; Badania defektow sieci krystalicznej metoda anihilacji pozytonow

    Energy Technology Data Exchange (ETDEWEB)

    Dryzek, J. [Institute of Nuclear Physics, Cracow (Poland)

    1994-12-31

    In this report the positrons annihilation methods as a tool for the crystal defects studies is presented. The short description of the positron - crystal interactions and different positron capture models are discussed. 192 refs, 67 figs, 6 tabs.

  5. Digitized detection of gamma-ray signals concentrated in narrow time windows for transient positron annihilation lifetime spectroscopy.

    Science.gov (United States)

    Kinomura, A; Suzuki, R; Oshima, N; O'Rourke, B E; Nishijima, T; Ogawa, H

    2014-12-01

    A pulsed slow-positron beam generated by an electron linear accelerator was directly used for positron annihilation lifetime spectroscopy without any positron storage devices. A waveform digitizer was introduced to simultaneously capture multiple gamma-ray signals originating from positron annihilation events during a single accelerator pulse. The positron pulse was chopped and bunched with the chopper signals also sent to the waveform digitizer. Time differences between the annihilation gamma-ray and chopper peaks were calculated and accumulated as lifetime spectra in a computer. The developed technique indicated that positron annihilation lifetime spectroscopy can be performed in a 20 μs time window at a pulse repetition rate synchronous with the linear accelerator. Lifetime spectra of a Kapton sheet and a thermally grown SiO2 layer on Si were successfully measured. Synchronization of positron lifetime measurements with pulsed ion irradiation was demonstrated by this technique.

  6. Gamma-ray Background Spectrum and Annihilation Rate in the Baryon-symmetric Big-bang Cosmology

    Science.gov (United States)

    Puget, J. L.

    1973-01-01

    An attempt was made to acquire experimental information on the problem of baryon symmetry on a large cosmological scale by observing the annihilation products. Data cover absorption cross sections and background radiation due to other sources for the two main products of annihilation, gamma rays and neutrinos. Test results show that the best direct experimental test for the presence of large scale antimatter lies in the gamma ray background spectrum between 1 and 70 MeV.

  7. Intrinsic spatial resolution limitations due to differences between positron emission position and annihilation detection localization

    International Nuclear Information System (INIS)

    Perez, Pedro; Malano, Francisco; Valente, Mauro

    2012-01-01

    Since its successful implementation for clinical diagnostic, positron emission tomography (PET) represents the most promising medical imaging technique. The recent major growth of PET imaging is mainly due to its ability to trace the biologic pathways of different compounds in the patient's body, assuming the patient can be labeled with some PET isotope. Regardless of the type of isotope, the PET imaging method is based on the detection of two 511-keV gamma photons being emitted in opposite directions, with almost 180 deg between them, as a consequence of electron-positron annihilation. Therefore, this imaging method is intrinsically limited by random uncertainties in spatial resolutions, related with differences between the actual position of positron emission and the location of the detected annihilation. This study presents an approach with the Monte Carlo method to analyze the influence of this effect on different isotopes of potential implementation in PET. (author)

  8. IceCube search for dark matter annihilation in nearby galaxies and galaxy clusters

    Science.gov (United States)

    Aartsen, M. G.; Abbasi, R.; Abdou, Y.; Ackermann, M.; Adams, J.; Aguilar, J. A.; Ahlers, M.; Altmann, D.; Auffenberg, J.; Bai, X.; Baker, M.; Barwick, S. W.; Baum, V.; Bay, R.; Beatty, J. J.; Bechet, S.; Becker Tjus, J.; Becker, K.-H.; Benabderrahmane, M. L.; BenZvi, S.; Berghaus, P.; Berley, D.; Bernardini, E.; Bernhard, A.; Bertrand, D.; Besson, D. Z.; Binder, G.; Bindig, D.; Bissok, M.; Blaufuss, E.; Blumenthal, J.; Boersma, D. J.; Bohaichuk, S.; Bohm, C.; Bose, D.; Böser, S.; Botner, O.; Brayeur, L.; Bretz, H.-P.; Brown, A. M.; Bruijn, R.; Brunner, J.; Carson, M.; Casey, J.; Casier, M.; Chirkin, D.; Christov, A.; Christy, B.; Clark, K.; Clevermann, F.; Coenders, S.; Cohen, S.; Cowen, D. F.; Cruz Silva, A. H.; Danninger, M.; Daughhetee, J.; Davis, J. C.; Day, M.; De Clercq, C.; De Ridder, S.; Desiati, P.; de Vries, K. D.; de With, M.; DeYoung, T.; Díaz-Vélez, J. C.; Dunkman, M.; Eagan, R.; Eberhardt, B.; Eisch, J.; Ellsworth, R. W.; Euler, S.; Evenson, P. A.; Fadiran, O.; Fazely, A. R.; Fedynitch, A.; Feintzeig, J.; Feusels, T.; Filimonov, K.; Finley, C.; Fischer-Wasels, T.; Flis, S.; Franckowiak, A.; Frantzen, K.; Fuchs, T.; Gaisser, T. K.; Gallagher, J.; Gerhardt, L.; Gladstone, L.; Glüsenkamp, T.; Goldschmidt, A.; Golup, G.; Gonzalez, J. G.; Goodman, J. A.; Góra, D.; Grandmont, D. T.; Grant, D.; Groß, A.; Ha, C.; Haj Ismail, A.; Hallen, P.; Hallgren, A.; Halzen, F.; Hanson, K.; Heereman, D.; Heinen, D.; Helbing, K.; Hellauer, R.; Hickford, S.; Hill, G. C.; Hoffman, K. D.; Hoffmann, R.; Homeier, A.; Hoshina, K.; Huelsnitz, W.; Hulth, P. O.; Hultqvist, K.; Hussain, S.; Ishihara, A.; Jacobi, E.; Jacobsen, J.; Jagielski, K.; Japaridze, G. S.; Jero, K.; Jlelati, O.; Kaminsky, B.; Kappes, A.; Karg, T.; Karle, A.; Kelley, J. L.; Kiryluk, J.; Kläs, J.; Klein, S. R.; Köhne, J.-H.; Kohnen, G.; Kolanoski, H.; Köpke, L.; Kopper, C.; Kopper, S.; Koskinen, D. J.; Kowalski, M.; Krasberg, M.; Krings, K.; Kroll, G.; Kunnen, J.; Kurahashi, N.; Kuwabara, T.; Labare, M.; Landsman, H.; Larson, M. J.; Lesiak-Bzdak, M.; Leuermann, M.; Leute, J.; Lünemann, J.; Macías, O.; Madsen, J.; Maggi, G.; Maruyama, R.; Mase, K.; Matis, H. S.; McNally, F.; Meagher, K.; Merck, M.; Meures, T.; Miarecki, S.; Middell, E.; Milke, N.; Miller, J.; Mohrmann, L.; Montaruli, T.; Morse, R.; Nahnhauer, R.; Naumann, U.; Niederhausen, H.; Nowicki, S. C.; Nygren, D. R.; Obertacke, A.; Odrowski, S.; Olivas, A.; Omairat, A.; O'Murchadha, A.; Paul, L.; Pepper, J. A.; Pérez de los Heros, C.; Pfendner, C.; Pieloth, D.; Pinat, E.; Posselt, J.; Price, P. B.; Przybylski, G. T.; Rädel, L.; Rameez, M.; Rawlins, K.; Redl, P.; Reimann, R.; Resconi, E.; Rhode, W.; Ribordy, M.; Richman, M.; Riedel, B.; Rodrigues, J. P.; Rott, C.; Ruhe, T.; Ruzybayev, B.; Ryckbosch, D.; Saba, S. M.; Salameh, T.; Sander, H.-G.; Santander, M.; Sarkar, S.; Schatto, K.; Scheriau, F.; Schmidt, T.; Schmitz, M.; Schoenen, S.; Schöneberg, S.; Schönwald, A.; Schukraft, A.; Schulte, L.; Schulz, O.; Seckel, D.; Sestayo, Y.; Seunarine, S.; Shanidze, R.; Sheremata, C.; Smith, M. W. E.; Soldin, D.; Spiczak, G. M.; Spiering, C.; Stamatikos, M.; Stanev, T.; Stasik, A.; Stezelberger, T.; Stokstad, R. G.; Stößl, A.; Strahler, E. A.; Ström, R.; Sullivan, G. W.; Taavola, H.; Taboada, I.; Tamburro, A.; Tepe, A.; Ter-Antonyan, S.; Tešić, G.; Tilav, S.; Toale, P. A.; Toscano, S.; Unger, E.; Usner, M.; Vallecorsa, S.; van Eijndhoven, N.; Van Overloop, A.; van Santen, J.; Vehring, M.; Voge, M.; Vraeghe, M.; Walck, C.; Waldenmaier, T.; Wallraff, M.; Weaver, Ch.; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.; Wiebe, K.; Wiebusch, C. H.; Williams, D. R.; Wissing, H.; Wolf, M.; Wood, T. R.; Woschnagg, K.; Xu, D. L.; Xu, X. W.; Yanez, J. P.; Yodh, G.; Yoshida, S.; Zarzhitsky, P.; Ziemann, J.; Zierke, S.; Zoll, M.

    2013-12-01

    We present the results of a first search for self-annihilating dark matter in nearby galaxies and galaxy clusters using a sample of high-energy neutrinos acquired in 339.8 days of live time during 2009/10 with the IceCube neutrino observatory in its 59-string configuration. The targets of interest include the Virgo and Coma galaxy clusters, the Andromeda galaxy, and several dwarf galaxies. We obtain upper limits on the cross section as a function of the weakly interacting massive particle mass between 300 GeV and 100 TeV for the annihilation into bb¯, W+W-, τ+τ-, μ+μ-, and νν¯. A limit derived for the Virgo cluster, when assuming a large effect from subhalos, challenges the weakly interacting massive particle interpretation of a recently observed GeV positron excess in cosmic rays.

  9. Search for dark matter annihilations in the sun with the 79-string IceCube detector.

    Science.gov (United States)

    Aartsen, M G; Abbasi, R; Abdou, Y; Ackermann, M; Adams, J; Aguilar, J A; Ahlers, M; Altmann, D; Auffenberg, J; Bai, X; Baker, M; Barwick, S W; Baum, V; Bay, R; Beattie, K; Beatty, J J; Bechet, S; Becker Tjus, J; Becker, K-H; Bell, M; Benabderrahmane, M L; BenZvi, S; Berdermann, J; Berghaus, P; Berley, D; Bernardini, E; Bernhard, A; Bertrand, D; Besson, D Z; Bindig, D; Bissok, M; Blaufuss, E; Blumenthal, J; Boersma, D J; Bohaichuk, S; Bohm, C; Bose, D; Böser, S; Botner, O; Brayeur, L; Brown, A M; Bruijn, R; Brunner, J; Buitink, S; Carson, M; Casey, J; Casier, M; Chirkin, D; Christy, B; Clark, K; Clevermann, F; Cohen, S; Cowen, D F; Cruz Silva, A H; Danninger, M; Daughhetee, J; Davis, J C; De Clercq, C; De Ridder, S; Desiati, P; de Vries-Uiterweerd, G; de With, M; DeYoung, T; Díaz-Vélez, J C; Dreyer, J; Dunkman, M; Eagan, R; Eberhardt, B; Eisch, J; Ellsworth, R W; Engdegård, O; Euler, S; Evenson, P A; Fadiran, O; Fazely, A R; Fedynitch, A; Feintzeig, J; Feusels, T; Filimonov, K; Finley, C; Fischer-Wasels, T; Flis, S; Franckowiak, A; Franke, R; Frantzen, K; Fuchs, T; Gaisser, T K; Gallagher, J; Gerhardt, L; Gladstone, L; Glüsenkamp, T; Goldschmidt, A; Golup, G; Goodman, J A; Góra, D; Grant, D; Groß, A; Gurtner, M; Ha, C; Haj Ismail, A; Hallgren, A; Halzen, F; Hanson, K; Heereman, D; Heimann, P; Heinen, D; Helbing, K; Hellauer, R; Hickford, S; Hill, G C; Hoffman, K D; Hoffmann, R; Homeier, A; Hoshina, K; Huelsnitz, W; Hulth, P O; Hultqvist, K; Hussain, S; Ishihara, A; Jacobi, E; Jacobsen, J; Japaridze, G S; Jero, K; Jlelati, O; Kaminsky, B; Kappes, A; Karg, T; Karle, A; Kelley, J L; Kiryluk, J; Kislat, F; Kläs, J; Klein, S R; Köhne, J-H; Kohnen, G; Kolanoski, H; Köpke, L; Kopper, C; Kopper, S; Koskinen, D J; Kowalski, M; Krasberg, M; Kroll, G; Kunnen, J; Kurahashi, N; Kuwabara, T; Labare, M; Landsman, H; Larson, M J; Lesiak-Bzdak, M; Leute, J; Lünemann, J; Madsen, J; Maruyama, R; Mase, K; Matis, H S; McNally, F; Meagher, K; Merck, M; Mészáros, P; Meures, T; Miarecki, S; Middell, E; Milke, N; Miller, J; Mohrmann, L; Montaruli, T; Morse, R; Nahnhauer, R; Naumann, U; Niederhausen, H; Nowicki, S C; Nygren, D R; Obertacke, A; Odrowski, S; Olivas, A; Olivo, M; O'Murchadha, A; Paul, L; Pepper, J A; Pérez de los Heros, C; Pfendner, C; Pieloth, D; Pirk, N; Posselt, J; Price, P B; Przybylski, G T; Rädel, L; Rawlins, K; Redl, P; Resconi, E; Rhode, W; Ribordy, M; Richman, M; Riedel, B; Rodrigues, J P; Rott, C; Ruhe, T; Ruzybayev, B; Ryckbosch, D; Saba, S M; Salameh, T; Sander, H-G; Santander, M; Sarkar, S; Schatto, K; Scheel, M; Scheriau, F; Schmidt, T; Schmitz, M; Schoenen, S; Schöneberg, S; Schönherr, L; Schönwald, A; Schukraft, A; Schulte, L; Schulz, O; Seckel, D; Seo, S H; Sestayo, Y; Seunarine, S; Sheremata, C; Smith, M W E; Soiron, M; Soldin, D; Spiczak, G M; Spiering, C; Stamatikos, M; Stanev, T; Stasik, A; Stezelberger, T; Stokstad, R G; Stößl, A; Strahler, E A; Ström, R; Sullivan, G W; Taavola, H; Taboada, I; Tamburro, A; Ter-Antonyan, S; Tilav, S; Toale, P A; Toscano, S; Usner, M; van der Drift, D; van Eijndhoven, N; Van Overloop, A; van Santen, J; Vehring, M; Voge, M; Vraeghe, M; Walck, C; Waldenmaier, T; Wallraff, M; Wasserman, R; Weaver, Ch; Wellons, M; Wendt, C; Westerhoff, S; Whitehorn, N; Wiebe, K; Wiebusch, C H; Williams, D R; Wissing, H; Wolf, M; Wood, T R; Woschnagg, K; Xu, C; Xu, D L; Xu, X W; Yanez, J P; Yodh, G; Yoshida, S; Zarzhitsky, P; Ziemann, J; Zierke, S; Zilles, A; Zoll, M

    2013-03-29

    We have performed a search for muon neutrinos from dark matter annihilation in the center of the Sun with the 79-string configuration of the IceCube neutrino telescope. For the first time, the DeepCore subarray is included in the analysis, lowering the energy threshold and extending the search to the austral summer. The 317 days of data collected between June 2010 and May 2011 are consistent with the expected background from atmospheric muons and neutrinos. Upper limits are set on the dark matter annihilation rate, with conversions to limits on spin-dependent and spin-independent scattering cross sections of weakly interacting massive particles (WIMPs) on protons, for WIMP masses in the range 20-5000  GeV/c2. These are the most stringent spin-dependent WIMP-proton cross section limits to date above 35  GeV/c2 for most WIMP models.

  10. Surfaces of colloidal PbSe nanocrystals probed by thin-film positron annihilation spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Chai, L.; Schut, H.; Schaarenburg, L. C. van; Eijt, S. W. H., E-mail: S.W.H.Eijt@tudelft.nl [Department of Radiation, Radionuclides and Reactors, Faculty of Applied Sciences, Delft University of Technology, Mekelweg 15, NL-2629 JB Delft (Netherlands); Al-Sawai, W.; Barbiellini, B.; Bansil, A. [Physics Department, Northeastern University, Boston, Massachusetts 02115 (United States); Gao, Y. [Department of Chemical Engineering, Faculty of Applied Sciences, Delft University of Technology, Julianalaan 136, NL-2628 BL Delft (Netherlands); Kavli Institute of Nanoscience, Faculty of Applied Sciences, Delft University of Technology, Lorentzweg 1, NL-2628 CJ Delft (Netherlands); Houtepen, A. J. [Department of Chemical Engineering, Faculty of Applied Sciences, Delft University of Technology, Julianalaan 136, NL-2628 BL Delft (Netherlands); Mijnarends, P. E. [Department of Radiation, Radionuclides and Reactors, Faculty of Applied Sciences, Delft University of Technology, Mekelweg 15, NL-2629 JB Delft (Netherlands); Physics Department, Northeastern University, Boston, Massachusetts 02115 (United States); Huis, M. A. van [Kavli Institute of Nanoscience, Faculty of Applied Sciences, Delft University of Technology, Lorentzweg 1, NL-2628 CJ Delft (Netherlands); Ravelli, L.; Egger, W. [Institut für Angewandte Physik und Messtechnik, Universität der Bundeswehr München, Werner-Heisenberg-Weg 39, D-85579 Neubiberg (Germany); Kaprzyk, S. [Physics Department, Northeastern University, Boston, Massachusetts 02115 (United States); Academy of Mining and Metallurgy AGH, PL-30059 Kraków (Poland)

    2013-08-01

    Positron annihilation lifetime spectroscopy and positron-electron momentum density (PEMD) studies on multilayers of PbSe nanocrystals (NCs), supported by transmission electron microscopy, show that positrons are strongly trapped at NC surfaces, where they provide insight into the surface composition and electronic structure of PbSe NCs. Our analysis indicates abundant annihilation of positrons with Se electrons at the NC surfaces and with O electrons of the oleic ligands bound to Pb ad-atoms at the NC surfaces, which demonstrates that positrons can be used as a sensitive probe to investigate the surface physics and chemistry of nanocrystals inside multilayers. Ab initio electronic structure calculations provide detailed insight in the valence and semi-core electron contributions to the positron-electron momentum density of PbSe. Both lifetime and PEMD are found to correlate with changes in the particle morphology characteristic of partial ligand removal.

  11. Search for Two Omega Meson Decays of Charmonium Resonances Produced in Proton - Antiproton Annihilations

    Energy Technology Data Exchange (ETDEWEB)

    Kasper, Jason J. [Northwestern U.

    2002-01-01

    In Fermilab experiment E835 a search has been performed for two w(782) vector meson decays of charmonium produced via $p\\bar{p}$ annihilation. All states with even charge conjugation quantum number are theoretically accessible via $ww$. No charmonium signals were clearly visible. The large nonresonant continuum from fjp annihilation to ww was observed to be predominantly pseudoscalar. 903 upper limit confidence intervals were calculated for $B(\\eta_c \\to $ww$)$ assuming various phase shifts, $\\delta$, between the resonant and nonresonant $ww$ production giving a range from 0.543 for $\\delta$ = 180° to 18% for $\\delta$ = 0°. Upper limits on $B(\\bar{p}p \\to \\eta^{\\prime}_c$) x $B(\\eta^{\\prime}_c \\to ww$) are also given over a range of assumed masses and widths for the $\\eta^{\\prime}_c$.

  12. Limits on dark matter annihilation in the sun using the ANTARES neutrino telescope

    Directory of Open Access Journals (Sweden)

    S. Adrián-Martínez

    2016-08-01

    Full Text Available A search for muon neutrinos originating from dark matter annihilations in the Sun is performed using the data recorded by the ANTARES neutrino telescope from 2007 to 2012. In order to obtain the best possible sensitivities to dark matter signals, an optimisation of the event selection criteria is performed taking into account the background of atmospheric muons, atmospheric neutrinos and the energy spectra of the expected neutrino signals. No significant excess over the background is observed and 90% C.L. upper limits on the neutrino flux, the spin-dependent and spin-independent WIMP-nucleon cross-sections are derived for WIMP masses ranging from 50 GeV to 5 TeV for the annihilation channels WIMP+WIMP→bb¯,W+W− and τ+τ−.

  13. Interface detection in poly-ethylene terephthalate-metal laminates using variable energy positron annihilation

    International Nuclear Information System (INIS)

    Escobar Galindo, R.; Schut, H.; Veen, A. van; Rastogi, R.; Vellinga, W.P.; Meijer, H.E.H.

    2005-01-01

    Thin coatings of poly-ethylene terephthalate (PET) on metal ('laminates') have been studied with a variable energy positron annihilation technique. A correlation between PET crystallinity and the positron annihilation parameter S related to the free volume in the polymer is found. It is shown that buried interfaces in these systems may be detected provided the S parameter of the polymer coating is lower than that of the substrate and higher than that of the surface. Also it is found that large positron diffusion lengths in the substrate favour interface detection. Further, changes in S parameter of PET-metal laminates were measured during uniaxial deformation and shown to be in qualitative accordance with a very simple model description that accounts for changes in free volume in PET during plastic deformation as well as the area fraction of cracks occurring in the PET

  14. Gamma-ray signatures of annihilation to charged leptons in dark matter substructure

    International Nuclear Information System (INIS)

    Kistler, Matthew D.; Siegal-Gaskins, Jennifer M.

    2010-01-01

    Because of their higher concentrations and small internal velocities, Milky Way subhalos can be at least as important as the smooth halo in accounting for the GeV positron excess via dark matter annihilation. After showing how this can be achieved in various scenarios, including in Sommerfeld models, we demonstrate that, in this case, the diffuse inverse-Compton emission resulting from electrons and positrons produced in substructure leads to a nearly-isotropic signal close to the level of the isotropic GeV gamma-ray background seen by Fermi. Moreover, we show that HESS cosmic-ray electron measurements can be used to constrain multi-TeV internal bremsstrahlung gamma rays arising from annihilation to charged leptons.

  15. Point defects and precipitation phenomena in Cu-Zn-Al alloys. A study by positrons annihilation

    International Nuclear Information System (INIS)

    Romero, R.; Salgueiro, W.; Somoza, A.; Ahlers, M.H.

    1990-01-01

    Monocrystalline phase Cu-Zn-Al samples in phase β (derived from a bcc structure) were treated with different homogenization thermal treatments, isothermal annealing, and tempering at different time intervals. In this way, point defects are fixed and gamma phase precipitation is induced. The evolution of this technique's characteristic parameters was followed with positron annihilation temporal spectroscopy at room temperature. Owing to the extreme sensitivity of positrons to defects like vacancies, it is possible to study the migration of these defects in detail. It can be seen that the presence of precipitates within the matrix phase modifies the annihilation parameters. Results are discussed as a function of the standard model for positron trapping by defects. (Author). 9 refs., 4 figs

  16. Production of hyperfragments by antiprotons at rest annihilating on nuclei in nuclear photoemulsion

    International Nuclear Information System (INIS)

    Batusov, Yu.A.; Bunyatov, S.A.; Pontecorvo, G.B.

    1992-01-01

    Events have been observed, for the first time, of the production, departure and mesonic decay of the light hyperfragments Λ 3 H and Λ 4 H in the annihilation on the light (C, N, O, S)-nuclei of antiprotons stopping in nuclear photoemulsion. The lower limit of the production probability of Λ 3 H and Λ 4 H hyperfragments per single antiproton stopping in nuclear photoemulsion has been determined to be (6.1±3.5)x10 -4 . The charge exchange, on nucleons of the residual nucleus, of K - -mesons resulting from the annihilation process has been demonstrated to be the most probable mechanism of hyperfragment production. 17 refs.; 9 figs

  17. Resonant Compton cooling and annihilation line production in gamma-ray bursts

    Science.gov (United States)

    Preece, R. D.; Harding, A. K.

    1992-01-01

    Attention is given to a synchrotron self-Compton emission model for gamma-ray bursts which produces narrow annihilation features for a variety of field strengths, primary electron injection energies, and injection rates. In this model, primary electrons are injected and cooled by synchrotron emission in a strong, homogeneous magnetic field, resulting in a pair cascade. Multiple resonant scattering with cyclotron photons efficiently traps and cools pairs in the ground state to an average energy where the Compton energy loss rate is zero, which is in agreement with previous estimates of a Compton temperature. The particle distributions in the ground state are determined by numerically solving the Fokker-Planck equation in the steady state. In the case of isotropic injection of primary electrons, a significant narrow-line feature appears in the overall emission. In the case of beamed injection, the annihilation line is broadened to the extent that it would not be observable.

  18. Beam Diagnostics for Measurements of Antiproton Annihilation Cross Sections at Ultra-low Energy

    Directory of Open Access Journals (Sweden)

    Todoroki K.

    2014-03-01

    Full Text Available The ASACUSA (Atomic Spectroscopy And Collisions Using Slow Antiprotons collaboration of CERN is currently attempting to measure the antiproton-nucleus in-flight annihilation cross sections on thin target foils of C, Pd, and Pt at 130 keV of kinetic energy. The low-energy antiprotons were supplied by the Antiproton Decelerator (AD and a radio-frequency quadrupole decelerator. For this measurement, a beam profile monitor based on secondary electron emission was developed. Data from this monitor was used to ensure that antiprotons were precisely tuned to the position of an 80-mm-diameter experimental target, by measuring the spatial profile of 200-ns-long beam pulses containing 105 − 106 antiprotons with an active area of 40 mm × 40 mm and a spatial resolution of 4 mm. By using this monitor, we succeeded in finely tuning antiproton beams on the target, and observed some annihilation events originating from the target.

  19. Determination of phase transitions in a lyotropic liquid crystal by Positron Annihilation technique

    International Nuclear Information System (INIS)

    Castillo V, V.M.

    1994-01-01

    Positron annihilation technique was used to determine the phase transitions in a lyotropic liquid crystal, as a function of temperature. Seven different concentrations of the surfactant cetyldimethylethylammonium bromide, were studied. The liquid crystal studied consisted of a binary system, formed by the surfactant and water. Positron annihilation technique has a very high sensitivity toward changes in the microestructure, in condensed matter, this is useful in order to detect the temperatures at which phase transitions occur and the number of these, in a liquid crystalline system. Thus, phase transitions are related with changes occurred in the ortho-positronium parameters: lifetime (τ 3 ) and intensity of formation (I 3 ). Six different kinds of phases were detected in the system studied in a temperature range of 35 to 140 Centigrade degrees, those phases were: hexagonal, hexagonal-lamellae, lamellae, lamellae-cubic, nematic and anisotropic. Using optical microscopic the textures of these phases were assigned. (Author)

  20. Deuterium trapping at vacancy clusters in electron/neutron-irradiated tungsten studied by positron annihilation spectroscopy

    Science.gov (United States)

    Toyama, T.; Ami, K.; Inoue, K.; Nagai, Y.; Sato, K.; Xu, Q.; Hatano, Y.

    2018-02-01

    Deuterium trapping at irradiation-induced defects in tungsten, a candidate material for plasma facing components in fusion reactors, was revealed by positron annihilation spectroscopy. Pure tungsten was electron-irradiated (8.5 MeV at ∼373 K and to a dose of ∼1 × 10-3 dpa) or neutron-irradiated (at 573 K to a dose of ∼0.3 dpa), followed by post-irradiation annealing at 573 K for 100 h in deuterium gas of ∼0.1 MPa. In both cases of electron- or neutron-irradiation, vacancy clusters were found by positron lifetime measurements. In addition, positron annihilation with deuterium electrons was demonstrated by coincidence Doppler broadening measurements, directly indicating deuterium trapping at vacancy-type defects. This is expected to cause significant increase in deuterium retention in irradiated-tungsten.

  1. High Energy Electron Signals from Dark Matter Annihilation in the Sun

    Energy Technology Data Exchange (ETDEWEB)

    Schuster, Philip; /SLAC; Toro, Natalia; /Stanford U., ITP; Weiner, Neal; Yavin, Itay; /New York U., CCPP

    2012-04-09

    In this paper we discuss two mechanisms by which high energy electrons resulting from dark matter annihilations in or near the Sun can arrive at the Earth. Specifically, electrons can escape the sun if DM annihilates into long-lived states, or if dark matter scatters inelastically, which would leave a halo of dark matter outside of the sun. Such a localized source of electrons may affect the spectra observed by experiments with narrower fields of view oriented towards the sun, such as ATIC, differently from those with larger fields of view such as Fermi. We suggest a simple test of these possibilities with existing Fermi data that is more sensitive than limits from final state radiation. If observed, such a signal will constitute an unequivocal signature of dark matter.

  2. Surfaces of colloidal PbSe nanocrystals probed by thin-film positron annihilation spectroscopy

    Directory of Open Access Journals (Sweden)

    L. Chai

    2013-08-01

    Full Text Available Positron annihilation lifetime spectroscopy and positron-electron momentum density (PEMD studies on multilayers of PbSe nanocrystals (NCs, supported by transmission electron microscopy, show that positrons are strongly trapped at NC surfaces, where they provide insight into the surface composition and electronic structure of PbSe NCs. Our analysis indicates abundant annihilation of positrons with Se electrons at the NC surfaces and with O electrons of the oleic ligands bound to Pb ad-atoms at the NC surfaces, which demonstrates that positrons can be used as a sensitive probe to investigate the surface physics and chemistry of nanocrystals inside multilayers. Ab initio electronic structure calculations provide detailed insight in the valence and semi-core electron contributions to the positron-electron momentum density of PbSe. Both lifetime and PEMD are found to correlate with changes in the particle morphology characteristic of partial ligand removal.

  3. The study of defects in metallic alloys by positron annihilation spectroscopy

    International Nuclear Information System (INIS)

    Romero, R.; Salgueiro, W.; Somoza, A.

    1990-01-01

    Positron annihilation spectroscopy (PAS) has become in a very useful non destructive testing to the study of condensed matter. Specially, in the last two decades, with the advent of solid state detectors and high-resolution time spectrometers. The basic information obtained with PAS in solid-state physics is on electronic structure in free defect materials. However, positron annihilation techniques (lifetime, angular correlation and Doppler broadening) have been succesfully applied to study crystal lattice defects with lower-than-average electron density, such as vacancies, small vacancy clusters, etc.. In this sense, information about: vacancy formation and migration energies, dislocations, grain boundaries, solid-solid phase transformation and radiation damage was obtained. In this work the application of the positron lifetime technique to study the thermal effects on a fine-grained superplastic Al-Ca-Zn alloy and the quenched-in defects in monocrystals of β Cu-Zn-Al alloy for several quenching temperatures is shown. (Author) [es

  4. The application of CANDU neutron economy for the annihilation of the minor actinides

    International Nuclear Information System (INIS)

    Dastur, Adi; Gagnon, Nathalie

    1995-01-01

    A strategically indispensable role, comparable to the one of operating with natural uranium, is proposed for CANDU as an incentive to ensure future CANDU sales in an environment where enrichment and reprocessing technology are globally available. Because of their high neutron economy, CANDU reactors can operate with minimal fissile content and consequently at high neutron flux. This is especially so in the absence of uranium, i.e. when transuranic actinides are used as fuel. The low fissile requirement and the on-power refuelling capability of CANDU can be exploited to achieve a once-through cycle for actinide annihilation. This avoids recycling and refabrication costs and provides relatively high annihilation rates. In addition, CANDUs ability to operate without uranium and extract energy from the minor actinides makes it the ultimate resource conserver and gives it a unique role in sustainable energy growth. (author)

  5. Antiproton-proton annihilation into light neutral meson pairs within an effective meson theory

    Science.gov (United States)

    Wang, Ying; Bystritskiy, Yury M.; Ahmadov, Azad I.; Tomasi-Gustafsson, Egle

    2017-08-01

    Antiproton-proton annihilation into light neutral mesons in the few GeV energy domain is investigated in view of a global description of the existing data and predictions for future work at the Antiproton Annihilation at Darmstadt (PANDA) experiment at the Facility for Antiproton and Ion Research (FAIR). An effective meson model earlier developed, with mesonic and baryonic degrees of freedom in s , t , and u channels, is applied here to π0π0 production. Form factors with logarithmic s and t (u ) dependencies are applied. A fair agreement with the existing angular distributions is obtained. Applying SU(3) symmetry, it is straightforward to recover the angular distributions for π0η and η η production in the same energy range. A good agreement is generally obtained with all existing data.

  6. Exciton-exciton annihilation and relaxation pathways in semiconducting carbon nanotubes.

    Science.gov (United States)

    Chmeliov, Jevgenij; Narkeliunas, Jonas; Graham, Matt W; Fleming, Graham R; Valkunas, Leonas

    2016-01-21

    We present a thorough analysis of one- and two-color transient absorption measurements performed on single- and double-walled semiconducting carbon nanotubes. By combining the currently existing models describing exciton-exciton annihilation-the coherent and the diffusion-limited ones-we are able to simultaneously reproduce excitation kinetics following both E11 and E22 pump conditions. Our simulations revealed the fundamental photophysical behavior of one-dimensional coherent excitons and non-trivial excitation relaxation pathways. In particular, we found that after non-linear annihilation a doubly-excited exciton relaxes directly to its E11 state bypassing the intermediate E22 manifold, so that after excitation resonant with the E11 transition, the E22 state remains unpopulated. A quantitative explanation for the observed much faster excitation kinetics probed at E22 manifold, comparing to those probed at the E11 band, is also provided.

  7. Positron Annihilation and Complementary Studies of Copper Sandblasted with Alumina Particles at Different Pressures

    Directory of Open Access Journals (Sweden)

    Paweł Horodek

    2017-11-01

    Full Text Available Positron annihilation spectroscopy and complementary methods were used to detect changes induced by sandblasting of alumina particles at different pressures varying from 1 to 6 bar in pure well-annealed copper. The positron lifetime measurements revealed existence of dislocations and vacancy clusters in the adjoined surface layer. The presence of retained alumina particles in the copper at the depth below 50 µm was found in the SEM pictures and also in the annihilation line shape parameter profiles measured in the etching experiment. The profiles show us that the total depth of damaged zones induced by sandblasting of alumina particles ranges from 140 µm up to ca. 800 µm and it depends on the applied pressure. The work-hardening of the adjoined surface layer was found in the microhardness measurements at the cross-section of the sandblasted samples.

  8. Positron Annihilation and Complementary Studies of Copper Sandblasted with Alumina Particles at Different Pressures.

    Science.gov (United States)

    Horodek, Paweł; Siemek, Krzysztof; Dryzek, Jerzy; Wróbel, Mirosław

    2017-11-23

    Positron annihilation spectroscopy and complementary methods were used to detect changes induced by sandblasting of alumina particles at different pressures varying from 1 to 6 bar in pure well-annealed copper. The positron lifetime measurements revealed existence of dislocations and vacancy clusters in the adjoined surface layer. The presence of retained alumina particles in the copper at the depth below 50 µm was found in the SEM pictures and also in the annihilation line shape parameter profiles measured in the etching experiment. The profiles show us that the total depth of damaged zones induced by sandblasting of alumina particles ranges from 140 µm up to ca. 800 µm and it depends on the applied pressure. The work-hardening of the adjoined surface layer was found in the microhardness measurements at the cross-section of the sandblasted samples.

  9. Synthesis of triplet-triplet annihilation upconversion nanocapsules under protective conditions.

    Science.gov (United States)

    Katta, Kartheek; Busko, Dmitry; Avlasevich, Yuri; Muñoz-Espí, Rafael; Baluschev, Stanislav; Landfester, Katharina

    2015-06-01

    Triplet-triplet annihilation upconversion (TTA-UC) nanocapsules are synthesized under oxygen-protective conditions (i.e., complete darkness and argon atmosphere) by free-radical miniemulsion polymerization. These conditions help to exclude the oxidation of the emitter molecules caused by singlet oxygen, generated during the synthesis at daylight conditions and oxygen-rich environment. Subsequently, keeping all the other experimental conditions the same, samples synthesized at protective conditions demonstrate substantially increased UC efficiency. These experimental facts strongly support the hypothesis that posterior removing of oxygen from TTA-UC nanocapsules is not sufficient to obtain reproducible and sustainable UC results. The schematic representation shows the influence of sunlight on the formation of singlet oxygen and its effect on the triplet-triplet annihilation upconversion process. © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  10. A study of some properties for substituted Li-ferrite using positron annihilation lifetime technique

    Directory of Open Access Journals (Sweden)

    E. Hassan Aly

    2015-01-01

    Full Text Available Positron annihilation lifetime spectroscopy (PALS is used to investigate polycrystalline substituted Li-ferrite samples. The dray ceramic technique was used to prepare all investigated samples. The variation of positron annihilation parameters I1%, I2%, τ1, and τ2 has been demonstrated with porosity and the initial permeability against the ionic radii of substituted ions for Li ferrite. The grain size (G.S. increased with increasing the ionic radii of the substituted ions for Li-ferrite. The correlation between I2 and τ2 has opposite behavior with the ionic radii of the substituted ions. Whereas the correlation between I1 and τ1; has nearly the same behavior with the ionic radii of the substituted ions except for V and Gd samples. There is mostly a direct correlation between the electrical resistivity and I2 values except for Sm sample with increasing the ionic radii of substituted ions.

  11. Amplification of Circularly Polarized Luminescence through Triplet-Triplet Annihilation-Based Photon Upconversion.

    Science.gov (United States)

    Han, Jianlei; Duan, Pengfei; Li, Xianggao; Liu, Minghua

    2017-07-26

    Amplification of circularly polarized luminescence (CPL) is demonstrated in a triplet-triplet annihilation-based photon upconversion (TTA-UC) system. When chiral binaphthyldiamine acceptors are sensitized with an achiral Pt(II) octaethylporphine (PtOEP) in solution, upconverted circularly polarized luminescence (UC-CPL) were observed for the first time, in which the positive or negative circularly polarized emission could be obtained respectively, following the molecular chirality of the acceptors (R/S). More interestingly, one order of magnitude amplification of the dissymmetry factor g lum in UC-CPL was obtained in comparison with the normal promoted CPL. The multistep photophysical process of TTA-UC including triplet-triplet energy transfer (TTET) and triplet-triplet annihilation (TTA) have been suggested to enhance the UC-CPL, which provided a new strategy to design CPL materials with a higher dissymmetry factor.

  12. Annihilation electrogenerated chemiluminescence of mixed metal chelates in solution: modulating emission colour by manipulating the energetics

    Science.gov (United States)

    Kerr, Emily; Doeven, Egan H.; Bower, David J.; Donnelly, Paul S.; Connell, Timothy U.

    2015-01-01

    We demonstrate the mixed annihilation electrogenerated chemiluminescence of tris(2,2′-bipyridine)ruthenium(ii) with various cyclometalated iridium(iii) chelates. Compared to mixed ECL systems comprising organic luminophores, the absence of T-route pathways enables effective predictions of the observed ECL based on simple estimations of the exergonicity of the reactions leading to excited state production. Moreover, the multiple, closely spaced reductions and oxidations of the metal chelates provide the ability to finely tune the energetics and therefore the observed emission colour. Distinct emissions from multiple luminophores in the same solution are observed in numerous systems. The relative intensity of these emissions and the overall emission colour are dependent on the particular oxidized and reduced species selected by the applied electrochemical potentials. Finally, these studies offer insights into the importance of electronic factors in the question of whether the reduced or oxidized partner becomes excited in annihilation ECL. PMID:28694941

  13. Inclusive momentum and angular distributions from electron positron annihilation at √s = 3.0, 3.8, and 4.8 GeV

    International Nuclear Information System (INIS)

    Hollebeek, R.

    1975-05-01

    Inclusive features of multi-hadron final states produced in the annihilations of electrons and positrons are presented. Data were taken at the colliding beam machine, SPEAR, at center-of-mass energies 3.0 GeV, 3.8 GeV, and 4.8 GeV. Reaction products were detected in an approximately 20 m 3 collection of spark chambers and counters, cylindrically arranged, in an axial magnetic field of approximately 4 KG, around the e + e - intersection region. Distributions of single-particle momenta and production angle and two-particle correlations are presented and compared with dynamical models. The results are in disagreement with expectations based on the successful parton--quark model of hadron structure. No generally satisfactory interpretation is available. (U.S.)

  14. Relevance of slow positron beam research to astrophysical studies of positron interactions and annihilation in the interstellar medium

    International Nuclear Information System (INIS)

    Guessoum, N.; Jean, P.; Gillard, W.

    2006-01-01

    The processes undergone by positrons in the interstellar medium (ISM) from the moments of their birth to their annihilation are examined. Both the physics of the positron interactions with gases and solids (dust grains), and the physical conditions and characteristics of the environments where the processes of energy loss, positronium formation, and annihilation taking place, are reviewed. An explanation is given as to how all the relevant physical information are taken into account in order to calculate annihilation rates and spectra of the 511 keV emission for the various phases of the ISM; special attention is paid to positron interactions with dust and with polycyclic aromatic hydrocarbons. An attempt is made to show to what extent the interactions between positrons and interstellar dust grains are similar to laboratory experiments in which beams of slow positrons impinge upon solids and surfaces. Sample results are shown for the effect of dust grains on positron annihilation spectra in some phases of the ISM which, together with high resolution spectra measured by satellites, can be used to infer useful knowledge about the environment where the annihilation is predominantly taking place and ultimately about the birth place and history of positrons in the Galaxy. The important complementarity between work done by the astrophysical and the solid-state positron communities is strongly emphasized and specific experimental work is suggested which could assist the modeling of the interaction and annihilation of positrons in the ISM

  15. Implications of dynamical symmetry breaking for high energy experiments

    International Nuclear Information System (INIS)

    Ali, A.

    1981-06-01

    A scenario of dynamical symmetry breaking as an alternative to the canonical Higgs mechanism with elementary spin-O fields is described, and its implications for high energy experiments contrasted with those of the canonical theory. The potential role of e + e - annihilation physics in unravelling the nature of spontaneous symmetry breaking is emphasized. (orig.)

  16. First evidence for the annihilation decay mode $B^{+} \\to D_{s}^{+} \\phi$

    CERN Document Server

    Aaij, R; Adametz, A; Adeva, B; Adinolfi, M; Adrover, C; Affolder, A; Ajaltouni, Z; Albrecht, J; Alessio, F; Alexander, M; Ali, S; Alkhazov, G; Alvarez Cartelle, P; Alves Jr, A A; Amato, S; Amhis, Y; Anderlini, L; Anderson, J; Appleby, R B; Aquines Gutierrez, O; Archilli, F; Artamonov, A; Artuso, M; Aslanides, E; Auriemma, G; Bachmann, S; Back, J J; Baesso, C; Baldini, W; Barlow, R J; Barschel, C; Barsuk, S; Barter, W; Bates, A; Bauer, Th; Bay, A; Beddow, J; Bediaga, I; Belogurov, S; Belous, K; Belyaev, I; Ben-Haim, E; Benayoun, M; Bencivenni, G; Benson, S; Benton, J; Berezhnoy, A; Bernet, R; Bettler, M -O; van Beuzekom, M; Bien, A; Bifani, S; Bird, T; Bizzeti, A; Bjørnstad, P M; Blake, T; Blanc, F; Blanks, C; Blouw, J; Blusk, S; Bobrov, A; Bocci, V; Bondar, A; Bondar, N; Bonivento, W; Borghi, S; Borgia, A; Bowcock, T J V; Bozzi, C; Brambach, T; van den Brand, J; Bressieux, J; Brett, D; Britsch, M; Britton, T; Brook, N H; Brown, H; Büchler-Germann, A; Burducea, I; Bursche, A; Buytaert, J; Cadeddu, S; Callot, O; Calvi, M; Calvo Gomez, M; Camboni, A; Campana, P; Carbone, A; Carboni, G; Cardinale, R; Cardini, A; Carson, L; Carvalho Akiba, K; Casse, G; Cattaneo, M; Cauet, Ch; Charles, M; Charpentier, Ph; Chen, P; Chiapolini, N; Chrzaszcz, M; Ciba, K; Cid Vidal, X; Ciezarek, G; Clarke, P E L; Clemencic, M; Cliff, H V; Closier, J; Coca, C; Coco, V; Cogan, J; Cogneras, E; Collins, P; Comerma-Montells, A; Contu, A; Cook, A; Coombes, M; Corti, G; Couturier, B; Cowan, G A; Craik, D; Cunliffe, S; Currie, R; D'Ambrosio, C; David, P; David, P N Y; De Bonis, I; De Bruyn, K; De Capua, S; De Cian, M; De Miranda, J M; De Paula, L; De Simone, P; Decamp, D; Deckenhoff, M; Degaudenzi, H; Del Buono, L; Deplano, C; Derkach, D; Deschamps, O; Dettori, F; Di Canto, A; Dickens, J; Dijkstra, H; Diniz Batista, P; Domingo Bonal, F; Donleavy, S; Dordei, F; Dosil Suárez, A; Dossett, D; Dovbnya, A; Dupertuis, F; Dzhelyadin, R; Dziurda, A; Dzyuba, A; Easo, S; Egede, U; Egorychev, V; Eidelman, S; van Eijk, D; Eisenhardt, S; Ekelhof, R; Eklund, L; El Rifai, I; Elsasser, Ch; Elsby, D; Esperante Pereira, D; Falabella, A; Färber, C; Fardell, G; Farinelli, C; Farry, S; Fave, V; Fernandez Albor, V; Ferreira Rodrigues, F; Ferro-Luzzi, M; Filippov, S; Fitzpatrick, C; Fontana, M; Fontanelli, F; Forty, R; Francisco, O; Frank, M; Frei, C; Frosini, M; Furcas, S; Gallas Torreira, A; Galli, D; Gandelman, M; Gandini, P; Gao, Y; Garnier, J-C; Garofoli, J; Garosi, P; Garra Tico, J; Garrido, L; Gaspar, C; Gauld, R; Gersabeck, E; Gersabeck, M; Gershon, T; Ghez, Ph; Gibson, V; Gligorov, V V; Göbel, C; Golubkov, D; Golutvin, A; Gomes, A; Gordon, H; Grabalosa Gándara, M; Graciani Diaz, R; Granado Cardoso, L A; Graugés, E; Graziani, G; Grecu, A; Greening, E; Gregson, S; Grünberg, O; Gui, B; Gushchin, E; Guz, Yu; Gys, T; Hadjivasiliou, C; Haefeli, G; Haen, C; Haines, S C; Hall, S; Hampson, T; Hansmann-Menzemer, S; Harnew, N; Harnew, S T; Harrison, J; Harrison, P F; Hartmann, T; He, J; Heijne, V; Hennessy, K; Henrard, P; Hernando Morata, J A; van Herwijnen, E; Hicks, E; Hill, D; Hoballah, M; Hopchev, P; Hulsbergen, W; Hunt, P; Huse, T; Hussain, N; Hutchcroft, D; Hynds, D; Iakovenko, V; Ilten, P; Imong, J; Jacobsson, R; Jaeger, A; Jahjah Hussein, M; Jans, E; Jansen, F; Jaton, P; Jean-Marie, B; Jing, F; John, M; Johnson, D; Jones, C R; Jost, B; Kaballo, M; Kandybei, S; Karacson, M; Karbach, T M; Keaveney, J; Kenyon, I R; Kerzel, U; Ketel, T; Keune, A; Khanji, B; Kim, Y M; Kochebina, O; Komarov, V; Koopman, R F; Koppenburg, P; Korolev, M; Kozlinskiy, A; Kravchuk, L; Kreplin, K; Kreps, M; Krocker, G; Krokovny, P; Kruse, F; Kucharczyk, M; Kudryavtsev, V; Kvaratskheliya, T; La Thi, V N; Lacarrere, D; Lafferty, G; Lai, A; Lambert, D; Lambert, R W; Lanciotti, E; Lanfranchi, G; Langenbruch, C; Latham, T; Lazzeroni, C; Le Gac, R; van Leerdam, J; Lees, J -P; Lefèvre, R; Leflat, A; Lefrançois, J; Leroy, O; Lesiak, T; Li, Y; Li Gioi, L; Liles, M; Lindner, R; Linn, C; Liu, B; Liu, G; von Loeben, J; Lopes, J H; Lopez Asamar, E; Lopez-March, N; Lu, H; Luisier, J; Mac Raighne, A; Machefert, F; Machikhiliyan, I V; Maciuc, F; Maev, O; Magnin, J; Maino, M; Malde, S; Manca, G; Mancinelli, G; Mangiafave, N; Marconi, U; Märki, R; Marks, J; Martellotti, G; Martens, A; Martin, L; Martín Sánchez, A; Martinelli, M; Martinez Santos, D; Massafferri, A; Mathe, Z; Matteuzzi, C; Matveev, M; Maurice, E; Mazurov, A; McCarthy, J; McGregor, G; McNulty, R; Meissner, M; Merk, M; Merkel, J; Milanes, D A; Minard, M -N; Molina Rodriguez, J; Monteil, S; Moran, D; Morawski, P; Mountain, R; Mous, I; Muheim, F; Müller, K; Muresan, R; Muryn, B; Muster, B; Mylroie-Smith, J; Naik, P; Nakada, T; Nandakumar, R; Nasteva, I; Needham, M; Neufeld, N; Nguyen, A D; Nguyen-Mau, C; Nicol, M; Niess, V; Nikitin, N; Nikodem, T; Nomerotski, A; Novoselov, A; Oblakowska-Mucha, A; Obraztsov, V; Oggero, S; Ogilvy, S; Okhrimenko, O; Oldeman, R; Orlandea, M; Otalora Goicochea, J M; Owen, P; Pal, B K; Palano, A; Palutan, M; Panman, J; Papanestis, A; Pappagallo, M; Parkes, C; Parkinson, C J; Passaleva, G; Patel, G D; Patel, M; Patrick, G N; Patrignani, C; Pavel-Nicorescu, C; Pazos Alvarez, A; Pellegrino, A; Penso, G; Pepe Altarelli, M; Perazzini, S; Perego, D L; Perez Trigo, E; Pérez-Calero Yzquierdo, A; Perret, P; Perrin-Terrin, M; Pessina, G; Petridis, K; Petrolini, A; Phan, A; Picatoste Olloqui, E; Pie Valls, B; Pietrzyk, B; Pilař, T; Pinci, D; Playfer, S; Plo Casasus, M; Polci, F; Polok, G; Poluektov, A; Polycarpo, E; Popov, D; Popovici, B; Potterat, C; Powell, A; Prisciandaro, J; Pugatch, V; Puig Navarro, A; Qian, W; Rademacker, J H; Rakotomiaramanana, B; Rangel, M S; Raniuk, I; Rauschmayr, N; Raven, G; Redford, S; Reid, M M; dos Reis, A C; Ricciardi, S; Richards, A; Rinnert, K; Rives Molina, V; Roa Romero, D A; Robbe, P; Rodrigues, E; Rodriguez Perez, P; Rogers, G J; Roiser, S; Romanovsky, V; Romero Vidal, A; Rouvinet, J; Ruf, T; Ruiz, H; Sabatino, G; Saborido Silva, J J; Sagidova, N; Sail, P; Saitta, B; Salzmann, C; Sanmartin Sedes, B; Sannino, M; Santacesaria, R; Santamarina Rios, C; Santinelli, R; Santovetti, E; Sapunov, M; Sarti, A; Satriano, C; Satta, A; Savrie, M; Schaack, P; Schiller, M; Schindler, H; Schleich, S; Schlupp, M; Schmelling, M; Schmidt, B; Schneider, O; Schopper, A; Schune, M -H; Schwemmer, R; Sciascia, B; Sciubba, A; Seco, M; Semennikov, A; Senderowska, K; Sepp, I; Serra, N; Serrano, J; Seyfert, P; Shapkin, M; Shapoval, I; Shatalov, P; Shcheglov, Y; Shears, T; Shekhtman, L; Shevchenko, O; Shevchenko, V; Shires, A; Silva Coutinho, R; Skwarnicki, T; Smith, N A; Smith, E; Smith, M; Sobczak, K; Soler, F J P; Soomro, F; Souza, D; Souza De Paula, B; Spaan, B; Sparkes, A; Spradlin, P; Stagni, F; Stahl, S; Steinkamp, O; Stoica, S; Stone, S; Storaci, B; Straticiuc, M; Straumann, U; Subbiah, V K; Swientek, S; Szczekowski, M; Szczypka, P; Szumlak, T; T'Jampens, S; Teklishyn, M; Teodorescu, E; Teubert, F; Thomas, C; Thomas, E; van Tilburg, J; Tisserand, V; Tobin, M; Tolk, S; Tonelli, D; Topp-Joergensen, S; Torr, N; Tournefier, E; Tourneur, S; Tran, M T; Tsaregorodtsev, A; Tsopelas, P; Tuning, N; Ubeda Garcia, M; Ukleja, A; Urner, D; Uwer, U; Vagnoni, V; Valenti, G; Vazquez Gomez, R; Vazquez Regueiro, P; Vecchi, S; Velthuis, J J; Veltri, M; Veneziano, G; Vesterinen, M; Viaud, B; Videau, I; Vieira, D; Vilasis-Cardona, X; Visniakov, J; Vollhardt, A; Volyanskyy, D; Voong, D; Vorobyev, A; Vorobyev, V; Voss, H; Voß, C; Waldi, R; Wallace, R; Wandernoth, S; Wang, J; Ward, D R; Watson, N K; Webber, A D; Websdale, D; Whitehead, M; Wicht, J; Wiedner, D; Wiggers, L; Wilkinson, G; Williams, M P; Williams, M; Wilson, F F; Wishahi, J; Witek, M; Witzeling, W; Wotton, S A; Wright, S; Wu, S; Wyllie, K; Xie, Y; Xing, F; Xing, Z; Yang, Z; Young, R; Yuan, X; Yushchenko, O; Zangoli, M; Zavertyaev, M; Zhang, F; Zhang, L; Zhang, W C; Zhang, Y; Zhelezov, A; Zhong, L; Zvyagin, A

    2013-01-01

    Evidence for the hadronic annihilation decay mode $B^{+} \\to D_s^{+}\\phi$ is found with greater than $3\\sigma$ significance. The branching fraction and \\CP asymmetry are measured to be \\begin{eqnarray} \\mathcal{B}(B^{+} \\to D_s^{+}\\phi) &=& \\left(1.87^{\\,+1.25}_{\\,-0.73}\\,({\\rm stat}) \\pm 0.19\\, ({\\rm syst}) \\pm 0.32\\, ({\\rm norm})\\right) \\times 10^{-6}, \

  17. Precise tests of QCD in e{sup +}e{sup {minus}} annihilation

    Energy Technology Data Exchange (ETDEWEB)

    Burrows, P.N.

    1997-03-01

    A pedagogical review is given of precise tests of QCD in electron-positron annihilation. Emphasis is placed on measurements that have served to establish QCD as the correct theory of strong interactions, as well as measurements of the coupling parameter {alpha}{sub s}. An outlook is given for future important tests at a high-energy e{sup +}e{sup {minus}} collider.

  18. Mass Dependence of HBT Correlations in e+e- Annihilation II

    International Nuclear Information System (INIS)

    Bialas, A.; Kucharczyk, M.; Palka, H.; Zalewski, K.

    2001-01-01

    This paper continues the study of the consequences of the Bjorken-Gottfried hypothesis for the HBT parameters measured in e + e - annihilation. It is shown that introducing a natural cut-off for transverse momenta of emitted particles, one can describe the observed ratio of transverse and longitudinal HBT radii for pions without destroying the good description of the mass dependence of the HBT parameters for heavier particles. (author)

  19. Gravitational Perturbations as a Possible Cause for Instability in the Measurements of Positron Annihilation

    Directory of Open Access Journals (Sweden)

    Vikin B. P.

    2006-04-01

    Full Text Available The annihilation of positrons is measured in a wide range of studies in the field of physical chemistry. One of the problems in these studies is the instability of the results of measurements. As shown in our research, instability may result from the change of nonregistering gravitational effects related to alteration of the tidal forces upon the change of moon phases and the seasonal changes of the distance between the Earth and the Sun.

  20. On the role of neutrinos telescopes in the search for Dark Matter annihilations in the Sun

    Science.gov (United States)

    Fornengo, Nicolao; Masiero, Antonio; Queiroz, Farinaldo S.; Yaguna, Carlos E.

    2017-12-01

    The observation of GeV neutrinos coming from the Sun would be a clear signal of dark matter if neutrinos produced by cosmic rays interaction are an irreducible but suppressed background. Current neutrino detectors have so far failed to detect such a signal, however, and bounds from direct and indirect dark matter searches may significantly restrict the possibility of observing it in future experiments such as Hyper-Kamiokande or IceCube-Gen2. In this work we assess, in the light of current data and of expected experimental sensitivities, the prospects for the detection of a neutrino signal from dark matter annihilations in the Sun. To be as general as possible, equilibrium between the capture and the annihilation rates in the Sun is not assumed in our analysis; instead, the dark matter scattering and annihilation cross sections are taken as free and independent parameters. We consider capture via both spin-dependent and spin-independent interactions, and annihilations into three representative final states: bbar b, W^+W^-, and τ+τ-. We find that when the capture in the Sun is dominated by spin-independent interactions, current direct detection bounds already preclude the observation of a neutrino signal in future experiments. For capture via spin-dependent interactions, a strong complementarity is observed, over most of the parameter space, between future neutrino detectors and planned direct and indirect dark matter detection experiments, such as PICO-500 and CTA. In this case, we also identify some regions of the parameter space that can be probed, via the neutrino flux from the Sun, only by future neutrino experiments.

  1. Characterization of zeolite Y pastilles for the ortho-positronium annihilation studies

    International Nuclear Information System (INIS)

    Alvarado D, E.; Garcia S, I.; Cabral P, A.

    2008-01-01

    This paper presents the characterization of zeolite Y pastilles prior to their study by the Positronium Annihilation Lifetimes Spectroscopy. The characterization is the estimation of porosity, the determination of its purity and crystal size for X-ray diffraction, the determination of its morphology and particle size by scanning electron microscopy and its specific area by the Brunauer-Emmett-Teller method. Presenting the first lifetimes measurements of positronium in zeolites LTA and Y. (Author)

  2. Positron annihilation in low-temperature rare gases. II. Argon and neon

    International Nuclear Information System (INIS)

    Canter, K.F.; Roellig, L.O.

    1975-01-01

    Lifetime measurements of slow-positron and ortho-positronium (o-Ps) annihilation were made in argon and neon gases at room temperature and below. The argon experiments cover the temperature range 115 to 300 0 K and the density range 0.0356 to 0.0726 g/cm 3 (approximately equal to 20 to 40 amagat). The slow-positron spectra in argon exhibit a departure from free-positron annihilation below 200 0 K. The departure becomes more marked as the temperature is lowered. No deviation from free o-Ps pickoff annihilation is observed in argon at low temperatures. The neon measurements cover the temperature range 30 to 300 0 K and the density range 0.032 to 0.89 g/cm 3 (approximately equal to 35 to 980 amagat). No effect of temperature on the slow-positron spectra throughout the temperature and density ranges investigated in neon is observed. The spectra are very exponential with a corresponding decay rate which is temperature as well as time independent and is directly proportional to density over the ranges investigated. The o-Ps data are more eventful in that the o-Ps lifetime at near-liquid densities is approximately 20 nsec, a factor of nearly 4 greater than the value obtained using the pickoff-annihilation coefficient obtained at lower densities. This is evidence for positronium-induced cavities in low-temperature neon. A brief discussion of the argon and neon results is given in the context of the explanations offered for the low-temperature effects observed in helium gas

  3. Probing dark matter decay and annihilation with Fermi LAT observations of nearby galaxy clusters

    International Nuclear Information System (INIS)

    Huang, Xiaoyuan; Vertongen, Gilles; Weniger, Christoph

    2011-09-01

    Galaxy clusters are promising targets for indirect dark matter searches. Gamma-ray signatures from the decay or annihilation of dark matter particles inside these clusters could be observable with the Fermi Large Area Telescope (LAT). Based on three years of Fermi LAT gamma-ray data, we analyze the flux coming from eight nearby clusters individually as well as in a combined likelihood analysis. Concentrating mostly on signals from dark matter decay, we take into account uncertainties of the cluster masses as determined by X-ray observations and model the cluster emission with extended sources. We do not find significant emission from any of the considered clusters and present limits on the dark matter lifetime and annihilation cross-section. We compare our lifetime limits derived from cluster observations with the limits that can be obtained from the extragalactic gamma-ray background, and find that in case of hadronic decay the cluster limits become competitive at dark matter masses below a few hundred GeV. Finally, we show that in presence of dark matter substructures down to 10 -6 solar masses the limits on the dark matter annihilation cross-section could improve by a factor of a few hundred, possibly going down to the thermal cross-section of 3 x 10 -26 cm 3 s -1 for dark matter masses < or similar 150 GeV and annihilation into b anti b. As a direct application of our results, we derive limits on the lifetime of gravitino dark matter in scenarios with R-parity violation. Implications of these limits for the possible observation of long-lived superparticles at the LHC are discussed. (orig.)

  4. Model-independent constraints on dark matter annihilation in dwarf spheroidal galaxies

    OpenAIRE

    Boddy, Kimberly; Kumar, Jason; Marfatia, Danny; Sandick, Pearl

    2018-01-01

    We present a general, model-independent formalism for determining bounds on the production of photons in dwarf spheroidal galaxies via dark matter annihilation, applicable to any set of assumptions about dark matter particle physics or astrophysics. As an illustration, we analyze gamma-ray data from the Fermi Large Area Telescope to constrain a variety of nonstandard dark matter models, several of which have not previously been studied in the context of dwarf galaxy searches.

  5. Probing dark matter decay and annihilation with Fermi LAT observations of nearby galaxy clusters

    Energy Technology Data Exchange (ETDEWEB)

    Huang, Xiaoyuan [Chinese Academy of Sciences, Beijing (China). National Astronomical Observatories; Max-Planck-Institut fuer Physik, Muenchen (Germany); Vertongen, Gilles [Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Institut d' Astrophysique de Paris, 75 - Paris (France); Weniger, Christoph [Max-Planck-Institut fuer Physik, Muenchen (Germany)

    2011-09-15

    Galaxy clusters are promising targets for indirect dark matter searches. Gamma-ray signatures from the decay or annihilation of dark matter particles inside these clusters could be observable with the Fermi Large Area Telescope (LAT). Based on three years of Fermi LAT gamma-ray data, we analyze the flux coming from eight nearby clusters individually as well as in a combined likelihood analysis. Concentrating mostly on signals from dark matter decay, we take into account uncertainties of the cluster masses as determined by X-ray observations and model the cluster emission with extended sources. We do not find significant emission from any of the considered clusters and present limits on the dark matter lifetime and annihilation cross-section. We compare our lifetime limits derived from cluster observations with the limits that can be obtained from the extragalactic gamma-ray background, and find that in case of hadronic decay the cluster limits become competitive at dark matter masses below a few hundred GeV. Finally, we show that in presence of dark matter substructures down to 10{sup -6} solar masses the limits on the dark matter annihilation cross-section could improve by a factor of a few hundred, possibly going down to the thermal cross-section of 3 x 10{sup -26} cm{sup 3}s{sup -1} for dark matter masses annihilation into b anti b. As a direct application of our results, we derive limits on the lifetime of gravitino dark matter in scenarios with R-parity violation. Implications of these limits for the possible observation of long-lived superparticles at the LHC are discussed. (orig.)

  6. Constraints on dark matter annihilation in clusters of galaxies with the Fermi large area telescope

    International Nuclear Information System (INIS)

    Ackermann, M.; Ajello, M.; Allafort, A.; Bechtol, K.; Blanford, R.D.; Bloom, E.D.; Borgland, A.W.; Bouvier, A.; Buehler, R.; Cameron, R.A.; Charles, E.; Chiang, J.; Claus, R.; Do Couto E Silva, E.; Drell, P.S.; Drlica-Wagner, A.; Dubois, R.; Edmonds, Y.; Glanzman, T.; Godfrey, G.; Hayashida, M.; Johannesson, G.; Johnson, A.S.; Kamae, T.; Lande, J.; Lee, S.H.; Madejski, G.M.; Michelson, P.F.; Mitthumsiri, W.; Monzani, M.E.; Moskalenko, I.V.; Murgia, S.; Nolan, P.L.; Omodei, N.; Panetta, J.H.; Porter, T.A.; Tanaka, T.; Thayer, J.B.; Thayer, J.G.; Waite, A.P.; Wang, P.; Baldini, L.; Bellazzini, R.; Bregeon, J.; Kuss, M.; Latronico, L.; Pesce-Rollins, M.; Razzano, M.; Sgro, C.; Spandre, G.; Ballet, J.; Casandjian, J.M.; Grenier, I.A.; Starck, J.L.; Tibaldo, L.

    2010-01-01

    Nearby clusters and groups of galaxies are potentially bright sources of high-energy gamma-ray emission resulting from the pair-annihilation of dark matter particles. However, no significant gamma-ray emission has been detected so far from clusters in the first 11 months of observations with the Fermi Large Area Telescope. We interpret this non-detection in terms of constraints on dark matter particle properties. In particular for leptonic annihilation final states and particle masses greater than similar to 200 GeV, gamma-ray emission from inverse Compton scattering of CMB photons is expected to dominate the dark matter annihilation signal from clusters, and our gamma-ray limits exclude large regions of the parameter space that would give a good fit to the recent anomalous Pamela and Fermi-LAT electron-positron measurements. We also present constraints on the annihilation of more standard dark matter candidates, such as the lightest neutralino of supersymmetric models. The constraints are particularly strong when including the fact that clusters are known to contain substructure at least on galaxy scales, increasing the expected gamma-ray flux by a factor of similar to 5 over a smooth-halo assumption. We also explore the effect of uncertainties in cluster dark matter density profiles, finding a systematic uncertainty in the constraints of roughly a factor of two, but similar overall conclusions. In this work, we focus on deriving limits on dark matter models; a more general consideration of the Fermi-LAT data on clusters and clusters as gamma-ray sources is forthcoming. (authors)

  7. On the possibility of universal interstitial emission induced annihilation in metallic nanostructures

    Science.gov (United States)

    Li, Xiangyan; Xu, Yichun; Duan, Guohua; Sun, Jingjing; Hao, Congyu; Zhang, Yange; Liu, Wei; Liu, C. S.; Fang, Q. F.

    2018-03-01

    Nano-structured metals have been explored as self-healing materials for radiation damage due to vacancy-interstitial recombination at interfaces, such as grain boundaries (GBs) in nanocrystals (NCs) and free surfaces in nanoporous metals (NPs). The annihilation in copper was recently proposed to be via the interstitial-emission (IE) from the GB. However, whether the IE is applied as a possibly universal mechanism in other NPs and NCs deserves further investigation. The interstitial is often considered to overcome a large binding energy with the GB/surface to migrate out of the GB/surface and induce annihilation. In this work, with emphasis on the IE in tungsten where the interstitial is exceptionally tightly bound to the tungsten GB/surface, we found that the interstitial only needed to migrate over a small distance from the GB/surface to recombine with the vacancy nearby at a small energy barrier. During the process, the annihilation region around a static interstitial at the GB/surface propagated or extended greatly to the adjacent bulk area. The annihilation was found to be via the IE from the GB/surface or coupled vacancy hop with the IE. The ratio of the interstitial-GB/surface binding energy to the trapping-radius of the GB/surface for the interstitial was proposed to be a better qualitative indicator for the difficulty in the IE than the binding energy. Given that the IE works in the investigated NPs and NCs tungsten, iron and copper where the interstitials of distinct configurations bind with the GBs/surfaces at diverse levels, the IE mechanism may work universally in various nano-structured metals.

  8. Evolution of porosity in a Portland cement paste studied through positron annihilation lifetime spectroscopy

    International Nuclear Information System (INIS)

    Consolati, G.; Quasso, F.

    2003-01-01

    Positron annihilation lifetime spectroscopy experiments were carried out in an ordinary Portland cement paste characterized by a water-to-cement ratio w/c=0.8, in order to monitor the porosity of the paste. It was found that ortho-positronium intensity is a suitable quantity to this purpose, being sensitive to the amount of water contained in the pores. The experimental data show good agreement with the porosity calculated according to the Powers' thin filmsodel

  9. New leptons, quarks and leptoquarks in high energy e+e- annihilation

    International Nuclear Information System (INIS)

    Buchmueller, W.

    1992-01-01

    Extensions of the standard model predict new spin-1/2 and spin-0 particles which may be colour singlets or colour triplets. We study pair production and single production of these particles in e + e - annihilation at 500 GeV center-of-mass energy. With the projected NLC luminosity, in most cases the production of new particles with masses close to the kinematical limit will be possible. We also discuss properties of final states resulting from heavy neutrino decays. (orig.)

  10. Azimuthal asymmetry in inclusive hadron production by e+e- annihilation

    International Nuclear Information System (INIS)

    Schwitters, R.F.; Boyarski, A.M.; Breidenbach, M.; Bulos, F.; Feldman, G.J.; Hanson, G.; Hartill, D.L.; Jean-Marie, B.; Larsen, R.R.; Luke, D.; Luth, V.; Lynch, H.L.; Morehouse, C.C.; Paterson, J.M.; Perl, M.L.; Pun, T.P.; Rapidis, P.; Richter, B.; Tanenbaum, W.; Vannucci, F.; Pierre, F.M.; Abrams, G.S.; Chinowsky, W.; Friedberg, C.E.; Goldhaber, G.; Kadyk, J.A.; Litke, A.M.; Lulu, B.A.; Sadoulet, B.; Trilling, G.H.; Whitaker, J.S.; Winkelmann, F.C.; Wiss, J.E.

    1975-01-01

    We have observed an azimuthal asymmetry in inclusive hadron production by e + e - annihilation at the center-of-mass energy √s = 7.4 GeV. The asymmetry is caused by the polarization of the circulating beams in the storage ring and allows separate determination of the transverse and longitudinal structure functions. We find that transverse production dominates for x > 0.2 where x is the scaling variable 2p/√s

  11. Application of positron annihilation techniques to the study of micels and microemulsions

    International Nuclear Information System (INIS)

    Olea C, O.

    1981-01-01

    The molecular auto-association mechanisms in sodium-oleate-alcohol-alkane-water systems were studied, applying positron and positronium annihilation techniques. The effects of the different component structures of these systems and of their concentrations on the swelled micel formation process which eventually produce microemulsions, were also investigated. The influences studied were: a) co-surfactant (alcohol) hydrocarbon chain lengths, b) alkane (oil) hydrocarbon chain lengths, c) surfactant concentrations, and d) surfactant double link alkylic chains. (author)

  12. Defect evolution during annealing of deformed FeSi alloys studied by positron annihilation spectroscopy

    Science.gov (United States)

    Mostafa, K. M.; Cámara, F. González; Petrov, Roumen; Calvillo, P. Rodríguez; De Grave, E.; Segers, D.; Houbaert, Y.

    2011-04-01

    High silicon steel is widely used in electrical appliances. Alloying iron with silicon improves its magnetic performance. A silicon content up to 6.5 wt. % gives excellent magnetic properties such as high saturation magnetization, near zero magnetostriction and low iron loss in high frequencies. Their workability is greatly reduced by the appearance of ordered structures, namely B2 and D03, as soon as the Si content becomes higher than 3.5 wt. %. This limits the mass production by conventional rolling to this maximum percentage of Si. In this work a series of FeSi (7.5 wt. % Si) samples with different degrees of deformation are investigated with positron annihilation spectroscopy and optical microscopy (OM). The influence of annealing on the concentration of defects of different deformed FeSi alloys has been investigated by positron annihilation lifetime spectroscopy and Doppler broadening of the annihilation radiation. OM is used to investigate the microstructure of deformed samples before and after annealing. The values of the S parameter present a decrease for all studied FeSi alloys with the increase of the annealing temperature, being attributed to a decrease of the concentration of defects. A sudden increase of the S-parameter value at 600 °C was observed for all samples, which could be related to the change of the ordering of the FeSi alloys at that temperature. At 700 °C, the values of the S parameter decreased drastically and starting from 900 °C, they became constant. The microstructures of the alloys, investigated by OM, show that recrystallization is completed at 900 °C and the samples are mainly free of defects, which is in agreement with the positron annihilation lifetime data.

  13. An undergraduate laboratory study of the polarisation of annihilation photons using Compton scattering

    OpenAIRE

    Knights, Patrick; Ryburn, Finlay; Tungate, Garry; Nikolopoulos, Konstantinos

    2018-01-01

    An experiment for the advanced undergraduate laboratory which allows students to study the effect of photon polarisation in Compton scattering and to explore q\\ uantum entanglement is described. The quantum entangled photons are produced through electron-positron annihilation in the $S$-state, and their polarisations a\\ re analysed using the Compton scattering cross-section dependence on the photon polarisation. The equipment necessary for this experiment is available at a typ\\ ical undergrad...

  14. Photocatalytic Supramolecular Enantiodifferentiating Dimerization of 2-Anthracenecarboxylic Acid through Triplet-Triplet Annihilation.

    Science.gov (United States)

    Rao, Ming; Kanagaraj, Kuppusamy; Fan, Chunying; Ji, Jiecheng; Xiao, Chao; Wei, Xueqin; Wu, Wanhua; Yang, Cheng

    2018-03-16

    Visible-light-driven enantiodifferentiating photodimerization of 2-anthracenecarboxylic acid (AC) sensitized by Schiff base Pt(II) complex-grafted γ-cyclodextrins leads the first triplet-triplet annihilation-based catalytic photochirogenesis. The syn-head-to-tail (HT) photodimer 2 was achieved in up to 31.4% ee at 61.0% conversion in the presence of 0.5% equiv of the photocatalyst.

  15. Observation of annihilation radiation from the Galactic center - The point and ridge components

    Science.gov (United States)

    Gruber, D. E.; Briggs, M. S.

    1991-01-01

    The point-source and Galactic-ridge components of the 511-keV annihilation radiation from the Galactic center are evaluated with an all-sky map based on detection at 80 keV through 2 MeV. The point-source flux is shown to be significant at 95-percent confidence and to agree with those of other data, while the ridge component is consistent with measurements taken at 25-deg longitude.

  16. 'Void existence' as against 'annihilation existence': Differentiating two qualities in primitive mental states.

    Science.gov (United States)

    Valdarsky, Irit Hameiri

    2015-10-01

    This paper attempts to distil out a particular quality of psychic (non)existence, which I call here 'void existence', from the quality predominantly explored in the psychoanalytic discourse on primitive mental states, which I call 'annihilation existence'. Achieving this phenomenological differentiation may make it easier to identify and work through extreme states in the analytic situation, when the patient is under the dominance of 'void existence'. I suggest that it is, as it were, a one-dimensional existence, in an infinite contour-less void, lacking any substantial internal object, lacking any substantial sense of psychic and/or somatic occurrences, and lacking any live representation of this very state of being. Hence, it lacks distress and anxiety, as well as calmness and peace. One might say that it is the inorganic within the organic; a quality of non-alive-ness within life. 'Annihilation existence' is existence in a two- or three-dimensional hollowed world, with flat and/or partial representations of self and object, which attracts acute distress and annihilation anxiety. It is a sort of existence on the brink of non-life, on the brink of the void; where a sense of catastrophic danger is brought on by the never-ending potentiality of the annihilation's realization. Both these psychic qualities can be encapsulated within neurotic and personality disorders, and the dominance of each can serve as defence against the dominance of the other. The theoretical discussion is supported by excerpts from an analysis. Copyright © 2015 Institute of Psychoanalysis.

  17. Gravitational Perturbations as a Possible Cause for Instability in the Measurements of Positron Annihilation

    Directory of Open Access Journals (Sweden)

    Vikin B. P.

    2006-04-01

    Full Text Available The annihilation of positrons is measured in a wide range of studies in the field of physical chemistry [1, 2]. One of the problems in these studies is the instability of the results of measurements [3–5]. As shown in our research, instability may result from the change of nonregistering gravitational effects related to alteration of the tidal forces upon the change of moon phases and the seasonal changes of the distance between the Earth and the Sun.

  18. Properties of eμ events produced in e+--e- annihilation

    International Nuclear Information System (INIS)

    Perl, M.L.

    1975-11-01

    The properties of the eμ events in e + e - annihilation are described as well as the relation of those properties to various hypotheses as to the nature of the events. New evidence is also presented using improved muon--pion separation. Angular and momentum distributions and cross sections are discussed. The data are consistent with the production of pairs of new particles. 17 references

  19. Moessbauer and positron annihilation studies of structural modifications of hemoglobin in solution

    International Nuclear Information System (INIS)

    Oshtrakh, M.I.; Kopelyan, E.A.; Semionkin, V.A.

    1995-01-01

    Structural modifications of human adult oxyhemoglobin in concentrated solution were studied by Moessbauer and positron life-time spectroscopies. The effects of non-sterile degradation and irradiation by γ-rays were compared by both techniques. It was found that positron annihilation parameters were sensitive to the structural modifications of hemoglobin molecules in solution and could be related with the conformational states of hemoglobin. (author)15 refs.; 3 tabs

  20. A realistic assessment of the CTA sensitivity to dark matter annihilation

    Energy Technology Data Exchange (ETDEWEB)

    Silverwood, Hamish; Weniger, Christoph; Bertone, Gianfranco [GRAPPA, University of Amsterdam, Science Park 904, Amsterdam, 1098 XH The Netherlands (Netherlands); Scott, Pat, E-mail: h.g.m.silverwood@uva.nl, E-mail: c.weniger@uva.nl, E-mail: p.scott@imperial.ac.uk, E-mail: gf.bertone@gmail.com [Department of Physics, Imperial College London, Blackett Laboratory, Prince Consort Road, London, SW7 2AZ United Kingdom (United Kingdom)

    2015-03-01

    We estimate the sensitivity of the upcoming CTA gamma-ray observatory to DM annihilation at the Galactic centre, improving on previous analyses in a number of significant ways. First, we perform a detailed analyses of all backgrounds, including diffuse astrophysical emission for the first time in a study of this type. Second, we present a statistical framework for including systematic errors and estimate the consequent degradation in sensitivity. These errors may come from e.g. event reconstruction, Monte Carlo determination of the effective area or uncertainty in atmospheric conditions. Third, we show that performing the analysis on a set of suitably optimised regions of interest makes it possible to partially compensate for the degradation in sensitivity caused by systematics and diffuse emission. To probe dark matter with the canonical thermal annihilation cross-section, CTA systematics like non-uniform variations in acceptance over a single field of view must be kept below the 0.3% level, unless the dark matter density rises more steeply in the centre of the Galaxy than predicted by a typical Navarro-Frenk-White or Einasto profile. For a contracted r{sup −1.3} profile, and systematics at the 1% level, CTA can probe annihilation to b b-bar at the canonical thermal level for dark matter masses between 100 GeV and 10 TeV.

  1. Search for annihilating dark matter in the Sun with 3 years of IceCube data

    International Nuclear Information System (INIS)

    Aartsen, M.G.; Hill, G.C.; Robertson, S.; Wallace, A.; Whelan, B.J.; Ackermann, M.; Bernardini, E.; Blot, S.; Bretz, H.P.; Franckowiak, A.; Jacobi, E.; Karg, T.; Kintscher, T.; Kunwar, S.; Nahnhauer, R.; Satalecka, K.; Spiering, C.; Stasik, A.; Strotjohann, N.L.; Terliuk, A.; Usner, M.; Santen, J. van; Adams, J.; Aguilar, J.A.; Ansseau, I.; Heereman, D.; Meagher, K.; Meures, T.; O'Murchadha, A.; Pinat, E.; Raab, C.; Ahlers, M.; Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J.C.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Griffith, Z.; Halzen, F.; Hanson, K.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J.L.; Kheirandish, A.; Krueger, C.; Mancina, S.; McNally, F.; Merino, G.; Sabbatini, L.; Tobin, M.N.; Tosi, D.; Vandenbroucke, J.; Van Rossem, M.; Wandkowsky, N.; Wendt, C.; Westerhoff, S.; Wille, L.; Xu, D.L.; Ahrens, M.; Bohm, C.; Dumm, J.P.; Finley, C.; Flis, S.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.; Altmann, D.; Anton, G.; Gluesenkamp, T.; Katz, U.; Kittler, T.; Tselengidou, M.; Andeen, K.; Anderson, T.; Dunkman, M.; Eller, P.; Huang, F.; Keivani, A.; Lanfranchi, J.L.; Pankova, D.V.; Quinnan, M.; Tesic, G.; Weiss, M.J.; Archinger, M.; Baum, V.; Boeser, S.; Pino Rosendo, E. del; Lorenzo, V. di; Eberhardt, B.; Ehrhardt, T.; Foesig, C.C.; Koepke, L.; Krueckl, G.; Peiffer, P.; Sandroos, J.; Steuer, A.; Wiebe, K.; Argueelles, C.; Axani, S.; Collin, G.H.; Conrad, J.M.; Jones, B.J.P.; Moulai, M.; Auffenberg, J.; Bissok, M.; Glauch, T.; Haack, C.; Hansmann, T.; Konietz, R.; Leuermann, M.; Penek, Oe.; Raedel, L.; Reimann, R.; Rongen, M.; Schoenen, S.; Schumacher, L.; Stettner, J.; Vehring, M.; Vogel, E.; Wallraff, M.; Wickmann, S.; Wiebusch, C.H.; Bai, X.; Barwick, S.W.; Yodh, G.; Bay, R.; Filimonov, K.; Price, P.B.; Woschnagg, K.; Beatty, J.J.; Becker Tjus, J.; Bos, F.; Eichmann, B.; Kroll, M.; Mandelartz, M.; Schoeneberg, S.; Tenholt, F.; Becker, K.H.; Bindig, D.; Helbing, K.; Hickford, S.; Hoffmann, R.; Kopper, S.; Lauber, F.; Naumann, U.; Obertacke Pollmann, A.; Soldin, D.; BenZvi, S.; Cross, R.; Berley, D.; Blaufuss, E.; Cheung, E.; Felde, J.; Friedman, E.; Hellauer, R.; Hoffman, K.D.; Maunu, R.; Olivas, A.; Schmidt, T.; Song, M.; Sullivan, G.W.; Bernhard, A.; Coenders, S.; Huber, M.; Krings, K.; Resconi, E.; Turcati, A.; Besson, D.Z.; Binder, G.; Gerhardt, L.; Klein, S.R.; Miarecki, S.; Palczewski, T.; Tatar, J.; Boerner, M.; Fuchs, T.; Meier, M.; Menne, T.; Pieloth, D.; Rhode, W.; Ruhe, T.; Sandrock, A.; Schlunder, P.; Bose, D.; Dujmovic, H.; In, S.; Jeong, M.; Kang, W.; Kim, J.; Kim, M.; Rott, C.

    2017-01-01

    We present results from an analysis looking for dark matter annihilation in the Sun with the IceCube neutrino telescope. Gravitationally trapped dark matter in the Sun's core can annihilate into Standard Model particles making the Sun a source of GeV neutrinos. IceCube is able to detect neutrinos with energies >100 GeV while its low-energy infill array DeepCore extends this to >10 GeV. This analysis uses data gathered in the austral winters between May 2011 and May 2014, corresponding to 532 days of live time when the Sun, being below the horizon, is a source of up-going neutrino events, easiest to discriminate against the dominant background of atmospheric muons. The sensitivity is a factor of two to four better than previous searches due to additional statistics and improved analysis methods involving better background rejection and reconstructions. The resultant upper limits on the spin-dependent dark matter-proton scattering cross section reach down to 1.46 x 10 -5 pb for a dark matter particle of mass 500 GeV annihilating exclusively into τ + τ - particles. These are currently the most stringent limits on the spin-dependent dark matter-proton scattering cross section for WIMP masses above 50 GeV. (orig.)

  2. Positron annihilation characteristics of ODS and non-ODS EUROFER isochronally annealed

    International Nuclear Information System (INIS)

    Ortega, Y.; Castro, V. de; Monge, M.A.; Munoz, A.; Leguey, T.; Pareja, R.

    2008-01-01

    Yttrium oxide dispersion strengthened (ODS) and non-ODS EUROFER produced by mechanical alloying and hot isostatic pressing have been subjected to isochronal annealing up to 1523 K, and the evolution of the open-volume defects and their thermal stability have been investigated using positron lifetime and coincidence Doppler broadening (CDB) techniques. Transmission electron microscopy (TEM) observations have also been performed on the studied samples to verify the characteristics of the surviving defects after annealing at 1523 K. The CDB spectra of ODS EUROFER exhibit a characteristic signature that is attributed to positron annihilation in Ar-decorated cavities at the oxide particle/matrix interfaces. The variation of the positron annihilation parameters with the annealing temperature shows three stages: up to 623 K, between 823 and 1323 K, and above 1323 K. Three-dimensional vacancy clusters, or voids, are detected in either materials in as-HIPed condition and after annealing at T ≤ 623 K. In the temperature range 823-1323 K, these voids' growth and nucleation and the growth of other new species of voids take place. Above 1323 K, some unstable cavities start to anneal out, and cavities associated to oxide particles and other small precipitates survive to annealing at 1523 K. The TEM observations and the positron annihilation results indicate that these cavities should be decorated with Ar atoms absorbed during the mechanical alloying process

  3. Search for dark matter annihilation in the Galactic Center with IceCube-79

    Science.gov (United States)

    Aartsen, M. G.; Abraham, K.; Ackermann, M.; Adams, J.; Aguilar, J. A.; Ahlers, M.; Ahrens, M.; Altmann, D.; Anderson, T.; Archinger, M.; Arguelles, C.; Arlen, T. C.; Auffenberg, J.; Bai, X.; Barwick, S. W.; Baum, V.; Bay, R.; Beatty, J. J.; Becker Tjus, J.; Becker, K.-H.; Beiser, E.; BenZvi, S.; Berghaus, P.; Berley, D.; Bernardini, E.; Bernhard, A.; Besson, D. Z.; Binder, G.; Bindig, D.; Bissok, M.; Blaufuss, E.; Blumenthal, J.; Boersma, D. J.; Bohm, C.; Börner, M.; Bos, F.; Bose, D.; Böser, S.; Botner, O.; Braun, J.; Brayeur, L.; Bretz, H.-P.; Brown, A. M.; Buzinsky, N.; Casey, J.; Casier, M.; Cheung, E.; Chirkin, D.; Christov, A.; Christy, B.; Clark, K.; Classen, L.; Coenders, S.; Cowen, D. F.; Cruz Silva, A. H.; Daughhetee, J.; Davis, J. C.; Day, M.; de André, J. P. A. M.; De Clercq, C.; Dembinski, H.; De Ridder, S.; Desiati, P.; de Vries, K. D.; de Wasseige, G.; de With, M.; DeYoung, T.; Díaz-Vélez, J. C.; Dumm, J. P.; Dunkman, M.; Eagan, R.; Eberhardt, B.; Ehrhardt, T.; Eichmann, B.; Euler, S.; Evenson, P. A.; Fadiran, O.; Fahey, S.; Fazely, A. R.; Fedynitch, A.; Feintzeig, J.; Felde, J.; Filimonov, K.; Finley, C.; Fischer-Wasels, T.; Flis, S.; Fuchs, T.; Glagla, M.; Gaisser, T. K.; Gaior, R.; Gallagher, J.; Gerhardt, L.; Ghorbani, K.; Gier, D.; Gladstone, L.; Glüsenkamp, T.; Goldschmidt, A.; Golup, G.; Gonzalez, J. G.; Góra, D.; Grant, D.; Gretskov, P.; Groh, J. C.; Groß, A.; Ha, C.; Haack, C.; Haj Ismail, A.; Hallgren, A.; Halzen, F.; Hansmann, B.; Hanson, K.; Hebecker, D.; Heereman, D.; Helbing, K.; Hellauer, R.; Hellwig, D.; Hickford, S.; Hignight, J.; Hill, G. C.; Hoffman, K. D.; Hoffmann, R.; Holzapfel, K.; Homeier, A.; Hoshina, K.; Huang, F.; Huber, M.; Huelsnitz, W.; Hulth, P. O.; Hultqvist, K.; In, S.; Ishihara, A.; Jacobi, E.; Japaridze, G. S.; Jero, K.; Jurkovic, M.; Kaminsky, B.; Kappes, A.; Karg, T.; Karle, A.; Kauer, M.; Keivani, A.; Kelley, J. L.; Kemp, J.; Kheirandish, A.; Kiryluk, J.; Kläs, J.; Klein, S. R.; Kohnen, G.; Kolanoski, H.; Konietz, R.; Koob, A.; Köpke, L.; Kopper, C.; Kopper, S.; Koskinen, D. J.; Kowalski, M.; Krings, K.; Kroll, G.; Kroll, M.; Kunnen, J.; Kurahashi, N.; Kuwabara, T.; Labare, M.; Lanfranchi, J. L.; Larson, M. J.; Lesiak-Bzdak, M.; Leuermann, M.; Leuner, J.; Lünemann, J.; Madsen, J.; Maggi, G.; Mahn, K. B. M.; Maruyama, R.; Mase, K.; Matis, H. S.; Maunu, R.; McNally, F.; Meagher, K.; Medici, M.; Meli, A.; Menne, T.; Merino, G.; Meures, T.; Miarecki, S.; Middell, E.; Middlemas, E.; Miller, J.; Mohrmann, L.; Montaruli, T.; Morse, R.; Nahnhauer, R.; Naumann, U.; Niederhausen, H.; Nowicki, S. C.; Nygren, D. R.; Obertacke, A.; Olivas, A.; Omairat, A.; O'Murchadha, A.; Palczewski, T.; Paul, L.; Pepper, J. A.; Pérez de los Heros, C.; Pfendner, C.; Pieloth, D.; Pinat, E.; Posselt, J.; Price, P. B.; Przybylski, G. T.; Pütz, J.; Quinnan, M.; Rädel, L.; Rameez, M.; Rawlins, K.; Redl, P.; Reimann, R.; Relich, M.; Resconi, E.; Rhode, W.; Richman, M.; Richter, S.; Riedel, B.; Robertson, S.; Rongen, M.; Rott, C.; Ruhe, T.; Ruzybayev, B.; Ryckbosch, D.; Saba, S. M.; Sabbatini, L.; Sander, H.-G.; Sandrock, A.; Sandroos, J.; Sarkar, S.; Schatto, K.; Scheriau, F.; Schimp, M.; Schmidt, T.; Schmitz, M.; Schoenen, S.; Schöneberg, S.; Schönwald, A.; Schukraft, A.; Schulte, L.; Seckel, D.; Seunarine, S.; Shanidze, R.; Smith, M. W. E.; Soldin, D.; Spiczak, G. M.; Spiering, C.; Stahlberg, M.; Stamatikos, M.; Stanev, T.; Stanisha, N. A.; Stasik, A.; Stezelberger, T.; Stokstad, R. G.; Stößl, A.; Strahler, E. A.; Ström, R.; Strotjohann, N. L.; Sullivan, G. W.; Sutherland, M.; Taavola, H.; Taboada, I.; Ter-Antonyan, S.; Terliuk, A.; Tešić, G.; Tilav, S.; Toale, P. A.; Tobin, M. N.; Tosi, D.; Tselengidou, M.; Unger, E.; Usner, M.; Vallecorsa, S.; van Eijndhoven, N.; Vandenbroucke, J.; van Santen, J.; Vanheule, S.; Veenkamp, J.; Vehring, M.; Voge, M.; Vraeghe, M.; Walck, C.; Wallraff, M.; Wandkowsky, N.; Weaver, Ch.; Wendt, C.; Westerhoff, S.; Whelan, B. J.; Whitehorn, N.; Wichary, C.; Wiebe, K.; Wiebusch, C. H.; Wille, L.; Williams, D. R.; Wissing, H.; Wolf, M.; Wood, T. R.; Woschnagg, K.; Xu, D. L.; Xu, X. W.; Xu, Y.; Yanez, J. P.; Yodh, G.; Yoshida, S.; Zarzhitsky, P.; Zoll, M.

    2015-10-01

    The Milky Way is expected to be embedded in a halo of dark matter particles, with the highest density in the central region, and decreasing density with the halo-centric radius. Dark matter might be indirectly detectable at Earth through a flux of stable particles generated in dark matter annihilations and peaked in the direction of the Galactic Center. We present a search for an excess flux of muon (anti-) neutrinos from dark matter annihilation in the Galactic Center using the cubic-kilometer-sized IceCube neutrino detector at the South Pole. There, the Galactic Center is always seen above the horizon. Thus, new and dedicated veto techniques against atmospheric muons are required to make the southern hemisphere accessible for IceCube. We used 319.7 live-days of data from IceCube operating in its 79-string configuration during 2010 and 2011. No neutrino excess was found and the final result is compatible with the background. We present upper limits on the self-annihilation cross-section, , for WIMP masses ranging from 30 GeV up to 10 TeV, assuming cuspy (NFW) and flat-cored (Burkert) dark matter halo profiles, reaching down to ˜eq 4 \\cdot 10^{-24} cm^3 s^{-1}, and ˜eq 2.6 \\cdot 10^{-23} cm^3 s^{-1} for the ν overline{ν } channel, respectively.

  4. Search for dark matter annihilation in the Galactic Center with IceCube-79

    Energy Technology Data Exchange (ETDEWEB)

    Aartsen, M.G.; Hill, G.C.; Robertson, S.; Whelan, B.J. [University of Adelaide, School of Chemistry and Physics, Adelaide, SA (Australia); Abraham, K.; Bernhard, A.; Coenders, S.; Gross, A.; Holzapfel, K.; Huber, M.; Jurkovic, M.; Krings, K.; Resconi, E.; Veenkamp, J. [Technische Universitaet Muenchen, Garching (Germany); Ackermann, M.; Berghaus, P.; Bernardini, E.; Bretz, H.P.; Cruz Silva, A.H.; Gluesenkamp, T.; Gora, D.; Jacobi, E.; Kaminsky, B.; Karg, T.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Schoenwald, A.; Shanidze, R.; Spiering, C.; Stasik, A.; Stoessl, A.; Strotjohann, N.L.; Terliuk, A.; Usner, M.; Yanez, J.P. [DESY, Zeuthen (Germany); Adams, J.; Brown, A.M. [University of Canterbury, Department of Physics and Astronomy, Private Bag 4800, Christchurch (New Zealand); Aguilar, J.A.; Heereman, D.; Meagher, K.; Meures, T.; O' Murchadha, A.; Pinat, E. [Universite Libre de Bruxelles, Science Faculty CP230, Brussels (Belgium); Ahlers, M.; Arguelles, C.; Beiser, E.; BenZvi, S.; Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J.C.; Fadiran, O.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Halzen, F.; Hanson, K.; Hoshina, K.; Jero, K.; Karle, A.; Kelley, J.L.; Kheirandish, A.; McNally, F.; Merino, G.; Middlemas, E.; Morse, R.; Richter, S.; Sabbatini, L.; Tobin, M.N.; Tosi, D.; Vandenbroucke, J.; Van Santen, J.; Wandkowsky, N.; Weaver, C.; Wendt, C.; Westerhoff, S.; Whitehorn, N.; Wille, L. [Wisconsin IceCube Particle Astrophysics Center, University of Wisconsin, Department of Physics, Madison, WI (United States); Ahrens, M.; Bohm, C.; Dumm, J.P.; Finley, C.; Flis, S.; Hulth, P.O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M. [Oskar Klein Centre, Stockholm University, Department of Physics, Stockholm (Sweden); Altmann, D.; Classen, L.; Kappes, A.; Tselengidou, M. [Friedrich-Alexander-Universitaet Erlangen-Nuernberg, Erlangen Centre for Astroparticle Physics, Erlangen (Germany); Anderson, T.; Arlen, T.C.; Dunkman, M.; Eagan, R.; Groh, J.C.; Huang, F.; Keivani, A.; Lanfranchi, J.L.; Quinnan, M.; Smith, M.W.E.; Stanisha, N.A.; Tesic, G. [Pennsylvania State University, Department of Physics, University Park, PA (United States); Archinger, M.; Baum, V.; Boeser, S.; Eberhardt, B.; Ehrhardt, T.; Koepke, L.; Kroll, G.; Luenemann, J.; Sander, H.G.; Schatto, K.; Wiebe, K. [University of Mainz, Institute of Physics, Mainz (Germany); Auffenberg, J.; Bissok, M.; Blumenthal, J.; Glagla, M.; Gier, D.; Gretskov, P.; Haack, C.; Hansmann, B.; Hellwig, D.; Kemp, J.; Konietz, R.; Koob, A.; Leuermann, M.; Leuner, J.; Paul, L.; Puetz, J.; Raedel, L.; Reimann, R.; Rongen, M.; Schimp, M.; Schoenen, S.; Schukraft, A.; Stahlberg, M.; Vehring, M.; Wallraff, M.; Wichary, C.; Wiebusch, C.H. [RWTH Aachen University, III. Physikalisches Institut, Aachen (Germany); Bai, X. [South Dakota School of Mines and Technology, Physics Department, Rapid City, SD (United States); Barwick, S.W.; Yodh, G. [University of California, Department of Physics and Astronomy, Irvine, CA (United States); Bay, R.; Filimonov, K.; Price, P.B.; Woschnagg, K. [University of California, Department of Physics, Berkeley, CA (United States); Beatty, J.J. [Ohio State University, Department of Physics and Center for Cosmology and Astro-Particle Physics, Columbus, OH (United States); Ohio State University, Department of Astronomy, Columbus, OH (United States); Becker Tjus, J.; Bos, F.; Eichmann, B.; Fedynitch, A.; Kroll, M.; Saba, S.M.; Schoeneberg, S. [Ruhr-Universitaet Bochum, Fakultaet fuer Physik and Astronomie, Bochum (Germany); Becker, K.H.; Bindig, D.; Fischer-Wasels, T.; Helbing, K.; Hickford, S.; Hoffmann, R.; Klaes, J.; Kopper, S.; Naumann, U.; Obertacke, A.; Omairat, A.; Posselt, J.; Soldin, D. [University of Wuppertal, Department of Physics, Wuppertal (Germany); Berley, D.; Blaufuss, E.; Cheung, E.; Christy, B.; Felde, J.; Hellauer, R.; Hoffman, K.D.; Huelsnitz, W.; Maunu, R.; Olivas, A.; Redl, P.; Schmidt, T.; Sullivan, G.W.; Wissing, H. [University of Maryland, Department of Physics, College Park, MD (United States); Besson, D.Z. [University of Kansas, Department of Physics and Astronomy, Lawrence, KS (United States); Binder, G.; Gerhardt, L.; Ha, C.; Klein, S.R.; Miarecki, S. [University of California, Department of Physics, Berkeley, CA (United States); Lawrence Berkeley National Laboratory, Berkeley, CA (United States); Boersma, D.J.; Botner, O.; Euler, S.; Hallgren, A.; Collaboration: IceCube Collaboration; and others

    2015-10-15

    The Milky Way is expected to be embedded in a halo of dark matter particles, with the highest density in the central region, and decreasing density with the halo-centric radius. Dark matter might be indirectly detectable at Earth through a flux of stable particles generated in dark matter annihilations and peaked in the direction of the Galactic Center. We present a search for an excess flux of muon (anti-) neutrinos from dark matter annihilation in the Galactic Center using the cubic-kilometer-sized IceCube neutrino detector at the South Pole. There, the Galactic Center is always seen above the horizon. Thus, new and dedicated veto techniques against atmospheric muons are required to make the southern hemisphere accessible for IceCube. We used 319.7 live-days of data from IceCube operating in its 79-string configuration during 2010 and 2011. No neutrino excess was found and the final result is compatible with the background. We present upper limits on the self-annihilation cross-section, left angle σ{sub A} right angle, for WIMP masses ranging from 30 GeV up to 10 TeV, assuming cuspy (NFW) and flat-cored (Burkert) dark matter halo profiles, reaching down to ≅ 4 . 10{sup -24} cm{sup 3}s{sup -1}, and ≅ 2.6 . 10{sup -23} cm{sup 3}s{sup -1} for the νanti ν channel, respectively. (orig.)

  5. Positron annihilation lifetime study of extended defects in semiconductor glasses and polymers

    Energy Technology Data Exchange (ETDEWEB)

    Boyko, Olha [Department of Pediatric Dentistry, Danylo Halytsky Lviv National Medical University, Pekarska str. 69, 79010 Lviv (Ukraine); Shpotyuk, Yaroslav [Department of Optoelectronics and Information Technologies, Ivan Franko National University of Lviv, Dragomanova str. 50, 79005 Lviv (Ukraine); Lviv Scientific Research Institute of Materials, Scientific Research Company ' ' Carat' ' , Stryjska str. 202, 79031 Lviv (Ukraine); Filipecki, Jacek [Institute of Physics, Jan Dlugosz University in Czestochowa, Armii Krajowej al. 13/15, 42200 Czestochowa (Poland)

    2013-01-15

    The processes of atomic shrinkage in network-forming solids initiated by external influences are tested using technique of positron annihilation lifetime spectroscopy at the example of chalcogenide vitreous semiconductors of arsenic sulphide type and acrylic polymers for dental application. Two state positron trapping is shown to be responsible for atomic shrinkage in chalcogenide glasses, while mixed trapping and ortho-positronium decaying is character for volumetric densification and stress propagation in acrylic dental polymers. At the basis of the obtained results it is concluded that correct analysis of externally-induced shrinkage in polymer networks under consideration can be developed by using original positron lifetime data treatment algorithms to compensate defect-free bulk annihilation channel within two-state positron trapping model and account for an interbalance between simultaneously co-existing positron trapping and orth-positronium related decaying channels within mixed three-state positron annihilation model (copyright 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

  6. Positron Annihilation Spectroscopy of High Performance Polymer Films under CO2 Pressure

    Energy Technology Data Exchange (ETDEWEB)

    C.A. Quarles; John R. Klaehn; Eric S. Peterson; Jagoda M. Urban-Klaehn

    2010-08-01

    Positron annihilation Lifetime and Doppler broadening measurements are reported for six polymer films as a function of carbon dioxide absolute pressure ranging from 0 to 45 psi. Since the polymer films were thin and did not absorb all positrons, corrections were made in the lifetime analysis for the absorption of positrons in the positron source and sample holder using the Monte Carlo transport code MCNP. Different polymers are found to behave differently. Some polymers studied form positronium and some, such as the polyimide structures, do not. For those samples that form positronium an interpretation in terms of free volume is possible; for those that don’t form positronium, further work is needed to determine how best to describe the behavior in terms of the bulk positron annihilation parameters. Some polymers exhibit changes in positron lifetime and intensity under CO2 pressure which may be described by the Henry or Langmuir sorption models, while the positron response of other polymers is rather insensitive to the CO2 pressure. The results demonstrate the usefulness of positron annihilation spectroscopy in investigating the sorption of CO2 into various polymers at pressures up to about 3 atm.

  7. Search for annihilating dark matter in the Sun with 3 years of IceCube data

    Energy Technology Data Exchange (ETDEWEB)

    Aartsen, M.G.; Hill, G.C.; Robertson, S.; Wallace, A.; Whelan, B.J. [University of Adelaide, Department of Physics, Adelaide (Australia); Ackermann, M.; Bernardini, E.; Blot, S.; Bretz, H.P.; Franckowiak, A.; Jacobi, E.; Karg, T.; Kintscher, T.; Kunwar, S.; Nahnhauer, R.; Satalecka, K.; Spiering, C.; Stasik, A.; Strotjohann, N.L.; Terliuk, A.; Usner, M.; Santen, J. van [DESY, Zeuthen (Germany); Adams, J. [University of Canterbury, Department of Physics and Astronomy, Private Bag 4800, Christchurch (New Zealand); Aguilar, J.A.; Ansseau, I.; Heereman, D.; Meagher, K.; Meures, T.; O' Murchadha, A.; Pinat, E.; Raab, C. [Universite Libre de Bruxelles, Science Faculty CP230, Brussels (Belgium); Ahlers, M.; Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J.C.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Griffith, Z.; Halzen, F.; Hanson, K.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J.L.; Kheirandish, A.; Krueger, C.; Mancina, S.; McNally, F.; Merino, G.; Sabbatini, L.; Tobin, M.N.; Tosi, D.; Vandenbroucke, J.; Van Rossem, M.; Wandkowsky, N.; Wendt, C.; Westerhoff, S.; Wille, L.; Xu, D.L. [University of Wisconsin, Department of Physics and Wisconsin IceCube Particle Astrophysics Center, Madison, WI (United States); Ahrens, M.; Bohm, C.; Dumm, J.P.; Finley, C.; Flis, S.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M. [Stockholm University, Department of Physics, Oskar Klein Centre, Stockholm (Sweden); Altmann, D.; Anton, G.; Gluesenkamp, T.; Katz, U.; Kittler, T.; Tselengidou, M. [Friedrich-Alexander-Universitaet Erlangen-Nuernberg, Erlangen Centre for Astroparticle Physics, Erlangen (Germany); Andeen, K. [Marquette University, Department of Physics, Milwaukee, WI (United States); Anderson, T.; Dunkman, M.; Eller, P.; Huang, F.; Keivani, A.; Lanfranchi, J.L.; Pankova, D.V.; Quinnan, M.; Tesic, G.; Weiss, M.J. [Pennsylvania State University, Department of Physics, University Park, PA (United States); Archinger, M.; Baum, V.; Boeser, S.; Pino Rosendo, E. del; Lorenzo, V. di; Eberhardt, B.; Ehrhardt, T.; Foesig, C.C.; Koepke, L.; Krueckl, G.; Peiffer, P.; Sandroos, J.; Steuer, A.; Wiebe, K. [University of Mainz, Institute of Physics, Mainz (Germany); Argueelles, C.; Axani, S.; Collin, G.H.; Conrad, J.M.; Jones, B.J.P.; Moulai, M. [Massachusetts Institute of Technology, Department of Physics, Cambridge, MA (United States); Auffenberg, J.; Bissok, M.; Glauch, T.; Haack, C.; Hansmann, T.; Konietz, R.; Leuermann, M.; Penek, Oe.; Raedel, L.; Reimann, R.; Rongen, M.; Schoenen, S.; Schumacher, L.; Stettner, J.; Vehring, M.; Vogel, E.; Wallraff, M.; Wickmann, S.; Wiebusch, C.H. [RWTH Aachen University, III. Physikalisches Institut, Aachen (Germany); Bai, X. [South Dakota School of Mines and Technology, Physics Department, Rapid City, SD (United States); Barwick, S.W.; Yodh, G. [University of California, Department of Physics and Astronomy, Irvine, CA (United States); Bay, R.; Filimonov, K.; Price, P.B.; Woschnagg, K. [University of California, Department of Physics, Berkeley, CA (United States); Beatty, J.J. [Ohio State University, Department of Physics and Center for Cosmology and Astro-Particle Physics, Columbus, OH (United States); Ohio State University, Department of Astronomy, Columbus, OH (United States); Becker Tjus, J.; Bos, F.; Eichmann, B.; Kroll, M.; Mandelartz, M.; Schoeneberg, S.; Tenholt, F. [Ruhr-Universitaet Bochum, Fakultaet fuer Physik and Astronomie, Bochum (Germany); Becker, K.H.; Bindig, D.; Helbing, K.; Hickford, S.; Hoffmann, R.; Kopper, S.; Lauber, F.; Naumann, U.; Obertacke Pollmann, A.; Soldin, D. [University of Wuppertal, Department of Physics, Wuppertal (Germany); BenZvi, S.; Cross, R. [University of Rochester, Department of Physics and Astronomy, Rochester, NY (United States); Berley, D.; Blaufuss, E.; Cheung, E.; Felde, J.; Friedman, E.; Hellauer, R.; Hoffman, K.D.; Maunu, R.; Olivas, A.; Schmidt, T.; Song, M.; Sullivan, G.W. [University of Maryland, Department of Physics, College Park, MD (United States); Bernhard, A.; Coenders, S.; Huber, M.; Krings, K.; Resconi, E.; Turcati, A. [Technische Universitaet Muenchen, Physik-Department, Garching (Germany); Besson, D.Z. [University of Kansas, Department of Physics and Astronomy, Lawrence, KS (United States); Binder, G.; Gerhardt, L.; Klein, S.R.; Miarecki, S.; Palczewski, T.; Tatar, J. [University of California, Department of Physics, Berkeley, CA (United States); Lawrence Berkeley National Laboratory, Berkeley, CA (United States); Boerner, M.; Fuchs, T.; Meier, M.; Menne, T.; Pieloth, D.; Rhode, W.; Ruhe, T.; Sandrock, A.; Schlunder, P. [TU Dortmund University, Department of Physics, Dortmund (Germany); Bose, D.; Dujmovic, H.; In, S.; Jeong, M.; Kang, W.; Kim, J.; Kim, M.; Rott, C. [Sungkyunkwan University, Department of Physics, Suwon (Korea, Republic of); Collaboration: IceCube Collaboration; and others

    2017-03-15

    We present results from an analysis looking for dark matter annihilation in the Sun with the IceCube neutrino telescope. Gravitationally trapped dark matter in the Sun's core can annihilate into Standard Model particles making the Sun a source of GeV neutrinos. IceCube is able to detect neutrinos with energies >100 GeV while its low-energy infill array DeepCore extends this to >10 GeV. This analysis uses data gathered in the austral winters between May 2011 and May 2014, corresponding to 532 days of live time when the Sun, being below the horizon, is a source of up-going neutrino events, easiest to discriminate against the dominant background of atmospheric muons. The sensitivity is a factor of two to four better than previous searches due to additional statistics and improved analysis methods involving better background rejection and reconstructions. The resultant upper limits on the spin-dependent dark matter-proton scattering cross section reach down to 1.46 x 10{sup -5} pb for a dark matter particle of mass 500 GeV annihilating exclusively into τ{sup +}τ{sup -} particles. These are currently the most stringent limits on the spin-dependent dark matter-proton scattering cross section for WIMP masses above 50 GeV. (orig.)

  8. Positron annihilation lifetime study of extended defects in semiconductor glasses and polymers

    International Nuclear Information System (INIS)

    Boyko, Olha; Shpotyuk, Yaroslav; Filipecki, Jacek

    2013-01-01

    The processes of atomic shrinkage in network-forming solids initiated by external influences are tested using technique of positron annihilation lifetime spectroscopy at the example of chalcogenide vitreous semiconductors of arsenic sulphide type and acrylic polymers for dental application. Two state positron trapping is shown to be responsible for atomic shrinkage in chalcogenide glasses, while mixed trapping and ortho-positronium decaying is character for volumetric densification and stress propagation in acrylic dental polymers. At the basis of the obtained results it is concluded that correct analysis of externally-induced shrinkage in polymer networks under consideration can be developed by using original positron lifetime data treatment algorithms to compensate defect-free bulk annihilation channel within two-state positron trapping model and account for an interbalance between simultaneously co-existing positron trapping and orth-positronium related decaying channels within mixed three-state positron annihilation model (copyright 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

  9. X-Ray Lines from Dark Matter Annihilation at the keV Scale.

    Science.gov (United States)

    Brdar, Vedran; Kopp, Joachim; Liu, Jia; Wang, Xiao-Ping

    2018-02-09

    In 2014, several groups reported hints for a yet unidentified line in astrophysical x-ray signals from galaxies and galaxy clusters at an energy of 3.5 keV. While it is not unlikely that this line is simply a reflection of imperfectly modeled atomic transitions, it has renewed the community's interest in models of keV-scale dark matter, whose decay would lead to such a line. The alternative possibility of dark matter annihilation into monochromatic photons is far less explored, a lapse that we strive to amend in this Letter. More precisely, we introduce a novel model of fermionic dark matter χ with O(keV) mass, annihilating to a scalar state ϕ which in turn decays to photons, for instance via loops of heavy vectorlike fermions. The resulting photon spectrum is box shaped, but if χ and ϕ are nearly degenerate in mass, it can also resemble a narrow line. We discuss dark matter production via two different mechanisms-misalignment and freeze-in-which both turn out to be viable in vast regions of parameter space. We constrain the model using astrophysical x-ray data, and we demonstrate that, thanks to the velocity dependence of the annihilation cross section, it has the potential to reconcile the various observations of the 3.5 keV line. We finally argue that the model can easily avoid structure formation constraints on keV-scale dark matter.

  10. Characterizing free volumes and layer structures in polymeric membranes using slow positron annihilation spectroscopy

    International Nuclear Information System (INIS)

    Jean, Y C; Chen Hongmin; Awad, Somia; Zhang Sui; Chen Hangzheng; Lau, Cher Hon; Wang Huan; Li Fuyun; Chung, Tai-Shung; Lee, L James; Huang, James

    2011-01-01

    Positron annihilation spectroscopy coupled with a newly built slow positron beam at National University of Singapore has been used to study the free volume, pore, and depth profile (0 - 10 μm) in cellulose acetate polymeric membrane at the bottom and top sides of membranes for ionic separation in water purification applications. The S and R parameters from Doppler broadening energy of annihilation radiation representing free volumes (0.1-1 nm size) and pores (>1 nm-μm) as a function of depth have been analyzed into multilayers, i.e. skin dense, transition, and porous layers, respectively. The top side of membrane has large free volumes and pores and the bottom side has a skin dense layer, which plays a key role in membrane performance. Positron annihilation lifetime results provide additional information about free-volume size and distribution at the atomic and molecular scale in polymeric membrane systems. Doppler broadening energy and lifetime spectroscopies coupled with a variable mono-energy slow positron beam are sensitive and novel techniques for characterization of polymeric membrane in separation applications.

  11. The suppression of pulsar and gamma-ray burst annihilation lines by magnetic photon splitting

    Science.gov (United States)

    Baring, Matthew G.

    1993-01-01

    Neutron stars, relativistic and compact by nature, show great potential for the copious creation of electron-positron pairs in the magnetospheres; these rapidly cool, thermalize, and then annihilate. It is therefore expected that many neutron sources might display evidence of pair annihilation lines in the 400-500 keV range. It is shown that magnetic photon splitting, which operates effectively at these energies and in the enormous neutron star magnetic fields, can destroy an annihilation feature by absorbing line photons and reprocessing them to lower energies. In so doing, photon splitting creates a soft gamma-ray bump and a broad quasi-power-law contribution to the X-ray continuum, which is too flat to conflict with the observed X-ray paucity in gamma-ray bursts. The destruction of the line occurs in neutron stars with surface fields of 5 x 10 exp 12 G or maybe even less, depending on the size of the emission region.

  12. Cross sections for inelastic meson-meson scattering via quark-antiquark annihilation

    Science.gov (United States)

    Shen, Zhen-Yu; Xu, Xiao-Ming; Weber, H. J.

    2016-08-01

    We study inelastic meson-meson scattering that is governed by quark-antiquark annihilation and creation involving a quark and an antiquark annihilating into a gluon, and subsequently the gluon creating another quark-antiquark pair. The resultant hadronic reactions include for I =1 : π π →ρ ρ , K K ¯→K*K¯*, K K¯*→K*K¯*, K*K ¯→K*K¯*, as well as π π →K K ¯, π ρ →K K¯*, π ρ →K*K ¯, and K K ¯→ρ ρ . In each reaction, one or two Feynman diagrams are involved in the Born approximation. We derive formulas for the unpolarized cross section, the transition amplitude, and the transition potential for quark-antiquark annihilation and creation. The unpolarized cross sections for the reactions are calculated at six temperatures, and prominent temperature dependence is found. It is due to differences among mesonic temperature dependence in hadronic matter.

  13. Positron annihilation spectroscopy study on annealing effect of CuO nanoparticles

    Energy Technology Data Exchange (ETDEWEB)

    Shi, Jianjian; Wang, Jiaheng; Yang, Wei; Zhu, Zhejie; Wu, Yichu, E-mail: ycwu@whu.edu.cn [School of Physics and Technology, Hubei Key Laboratory of Nuclear Solid State Physics, Wuhan University (WHU), Wuhan (China)

    2016-03-15

    The microstructure and defects of CuO nanoparticles under isochronal annealing were investigated by positron annihilation spectroscopy (PAS), X-ray diffraction (XRD) and scanning electron microscope (SEM). XRD and SEM results indicated that the average grain sizes of CuO nanoparticles grew slowly below 800 °C, and then increased rapidly with the annealing temperature from 800 to 1000 °C. Positron lifetime analysis exhibited that positrons were mainly annihilated in mono-vacancies (V{sub Cu}, V{sub O}) and vacancy clusters when annealing from 200 to 800 °C. Furthermore, W-S plot of Doppler broadening spectra at different annealing temperatures found that the (W, S) points distributed on two different defect species, which suggested that V{sup −}{sub Cu} - V{sup +}{sub O} complexes were produced when the grains grew to bigger size after annealing above 800 °C, and positrons might annihilate at these complexes. (author)

  14. Weak annihilation and new physics in charmless B → MM decays

    Energy Technology Data Exchange (ETDEWEB)

    Bobeth, Christoph [Institute for Advanced Study, Technische Universitaet Muenchen, Garching (Germany); Gorbahn, Martin [University of Liverpool, Department of Mathematical Sciences, Liverpool (United Kingdom); Vickers, Stefan [Excellence Cluster Universe, Technische Universitaet Muenchen, Garching (Germany)

    2015-07-15

    We use currently available data of nonleptonic charmless 2-body B → MM decays (MM = PP, PV,VV) that are mediated by b → (d, s) QCD- and QED-penguin operators to study weak annihilation and new-physics effects in the framework of QCD factorization. In particular we introduce one weak-annihilation parameter for decays related by (u <-> d) quark interchange and test this universality assumption. Within the standard model, the data supports this assumption with the only exceptions in the B → Kπ system, which exhibits the well-known ''ΔA{sub CP} puzzle'', and some tensions in B → K*φ. Beyond the standard model, we simultaneously determine weak-annihilation and new-physics parameters from data, employing model independent scenarios that address the ''ΔA{sub CP} puzzle'', such as QED-penguins and b → s anti uu current-current operators. We discuss also possibilities that allow further tests of our assumption once improved measurements from LHCb and Belle II become available. (orig.)

  15. Extragalactic diffuse γ-rays from dark matter annihilation: revised prediction and full modelling uncertainties

    Science.gov (United States)

    Hütten, M.; Combet, C.; Maurin, D.

    2018-02-01

    Recent high-energy data from Fermi-LAT on the diffuse γ-ray background have been used to set among the best constraints on annihilating TeV cold dark matter candidates. In order to assess the robustness of these limits, we revisit and update the calculation of the isotropic extragalactic γ-ray intensity from dark matter annihilation. The emission from halos with masses >= 1010 Msolar provides a robust lower bound on the predicted intensity. The intensity including smaller halos whose properties are extrapolated from their higher mass counterparts is typically 5 times higher, and boost from subhalos yields an additional factor ~ 1.5. We also rank the uncertainties from all ingredients and provide a detailed error budget for them. Overall, our fiducial intensity is a factor 5 lower than the one derived by the Fermi-LAT collaboration in their latest analysis. This indicates that the limits set on extragalactic dark matter annihilations could be relaxed by the same factor. We also calculate the expected intensity for self-interacting dark matter in massive halos and find the emission reduced by a factor 3 compared to the collisionless counterpart. The next release of the CLUMPY code will provide all the tools necessary to reproduce and ease future improvements of this prediction.

  16. Gamma-ray spectra of hexane (C6H14) in positron-electron annihilation process

    Science.gov (United States)

    Ma, Xiaoguang; Wang, Feng

    2013-08-01

    Theoretical gamma-ray spectra of molecule hexane have been calculated and compared with the experimental results in both gas (Iwata et al., 1997a) and liquid (Kerr et al., 1965) phases. The present study reveals that in gas phase not all valence electrons of hexane contribute the same degree in the electron-positron annihilation of hexane. The electrons which dominate the positron-electron annihilation of molecules are called positrophilic electrons. The positrophilic electrons are predominately found to involve the electrons on the lowest occupied valence orbital (LOVO) of a free molecule in gas phase. When hexane is confined in liquid phase, however, the intermolecular interactions ultimately eliminate the free molecular orientation and selectivity for the positrophilic electrons in the gas phase. As a result, the gamma-ray spectra of hexane become an "averaged" contribution from all valence electrons, which is again in agreement with liquid phase measurement. The roles of valence electrons in annihilation process for gas and liquid phases of hexane have been recognized for the first time in the present study.

  17. Investigation of cation vacancies in Zinc substituted maghemite by positron annihilation lifetime and Doppler broadening spectroscopy.

    Science.gov (United States)

    Asgarian, S M; Kargar, Z; Mozaffari, M

    2017-07-01

    In this work we investigated vacancies in maghemite and Zn substituted maghemite (γ-Fe 2-y Zn 3y/2 O 3 , y=0.0, 0.11, 0.24, 0.36, 0.50 and 0.66) nanoparticles using coincidence Doppler broadening and positron annihilation lifetime spectroscopy. Coincidence Doppler broadening spectroscopy (CDBS) measurements showed that the positrons annihilated in cation vacancies that surrounded by oxygen anions. Also, the CDBS showed that in pure maghemite and in the y=0.11 samples the vacancies are in octahedral and tetrahedral sites, respectively. For other samples they are distributed in both octahedral and tetrahedral sites. The positron annihilation lifetime spectroscopy (PALS) measurements confirmed the results of the CDBS measurements and also exhibited that the number of vacancies in y=0.36 sample is less than the other samples. This is attributed to Zn substituted magnetite phase in this sample as well as Zn substituted maghemite phase. Copyright © 2017 Elsevier Ltd. All rights reserved.

  18. X-Ray Lines from Dark Matter Annihilation at the keV Scale

    Science.gov (United States)

    Brdar, Vedran; Kopp, Joachim; Liu, Jia; Wang, Xiao-Ping

    2018-02-01

    In 2014, several groups reported hints for a yet unidentified line in astrophysical x-ray signals from galaxies and galaxy clusters at an energy of 3.5 keV. While it is not unlikely that this line is simply a reflection of imperfectly modeled atomic transitions, it has renewed the community's interest in models of keV-scale dark matter, whose decay would lead to such a line. The alternative possibility of dark matter annihilation into monochromatic photons is far less explored, a lapse that we strive to amend in this Letter. More precisely, we introduce a novel model of fermionic dark matter χ with O (keV ) mass, annihilating to a scalar state ϕ which in turn decays to photons, for instance via loops of heavy vectorlike fermions. The resulting photon spectrum is box shaped, but if χ and ϕ are nearly degenerate in mass, it can also resemble a narrow line. We discuss dark matter production via two different mechanisms—misalignment and freeze-in—which both turn out to be viable in vast regions of parameter space. We constrain the model using astrophysical x-ray data, and we demonstrate that, thanks to the velocity dependence of the annihilation cross section, it has the potential to reconcile the various observations of the 3.5 keV line. We finally argue that the model can easily avoid structure formation constraints on keV-scale dark matter.

  19. Possible Dark Matter Annihilation Signal in the AMS-02 Antiproton Data.

    Science.gov (United States)

    Cui, Ming-Yang; Yuan, Qiang; Tsai, Yue-Lin Sming; Fan, Yi-Zhong

    2017-05-12

    Using the latest AMS-02 cosmic-ray antiproton flux data, we search for a potential dark matter annihilation signal. The background parameters about the propagation, source injection, and solar modulation are not assumed a priori but based on the results inferred from the recent B/C ratio and proton data measurements instead. The possible dark matter signal is incorporated into the model self-consistently under a Bayesian framework. Compared with the astrophysical background-only hypothesis, we find that a dark matter signal is favored. The rest mass of the dark matter particles is ∼20-80  GeV, and the velocity-averaged hadronic annihilation cross section is about (0.2-5)×10^{-26}  cm^{3} s^{-1}, in agreement with that needed to account for the Galactic center GeV excess and/or the weak GeV emission from dwarf spheroidal galaxies Reticulum 2 and Tucana III. Tight constraints on the dark matter annihilation models are also set in a wide mass region.

  20. Ageing phenomenon in acrylic polymer dental materials detected by means of positron annihilation lifetime spectroscopy.

    Science.gov (United States)

    Filipecki, Jacek; Chamerski, Kordian; Boyko, Olha; Kotynia, Katarzyna

    2014-01-01

    Polymer materials based on acrylic monomers are commonly used in dentistry. It is important to research the structure of dental filling materials towards the material ageing. The study has been conducted in order to determine the presence of free volume gaps in the structure of polymer materials. Brand new, acrylic polymer based samples of dental Dipol materials were used as a research material. The study was conducted by means of the positron annihilation lifetime spectroscopy (PALS). As a result of the conducted measurements, curves describing numbers of counts of the acts of annihilation in the time function were obtained. The conducted studies revealed the existence of four components τ1, τ2, τ3 and τ4. The τ3 and τ4 components are attributed to the pick-off annihilation of o-Ps orthopositronium trapping by free volume gaps and provide information about geometrical parameters of the volumes. LT 9 computer program was used to calculate components. Free volume holes were determined from empirical relationship between the radius of free volume and the long lifetime components. Conducted studies indicate the presence of free volume holes in the research materials. It has been noted that a new long lifetime component is assigned to a new kind of free volumes that exist in the structure of material related to the material ageing.