WorldWideScience

Sample records for attosecond electron pulses

  1. Spatial transport of electron quantum states with strong attosecond pulses

    Science.gov (United States)

    Chovancova, M.; Agueny, H.; Førre, M.; Kocbach, L.; Hansen, J. P.

    2017-11-01

    This work follows up the work of Dimitrovsky, Briggs and co-workers on translated electron atomic states by a strong field of an atto-second laser pulse, also described as creation of atoms without a nucleus. Here, we propose a new approach by analyzing the electron states in the Kramers–Henneberger moving frame in the dipole approximation. The wave function follows the displacement vector α (t). This allows arbitrarily shaped pulses, including the model delta-function potentials in the Dimitrovsky and Briggs approach. In the case of final-length single-cycle pulses, we apply both the Kramers–Henneberger moving frame analysis and a full numerical treatment of our 1D model. When the laser pulse frequency exceeds the frequency associated by the energy difference between initial and final states, the entire wavefunction is translated in space nearly without loss of coherence, to a well defined distance from the original position where the ionized core is left behind. This statement is demonstrated on the excited Rydberg states (n = 10, n = 15), where almost no distortion in the transported wave functions has been observed. However, the ground state (n = 1) is visibly distorted during the removal by pulses of reasonable frequencies, as also predicted by Dimitrovsky and Briggs analysis. Our approach allows us to analyze general pulses as well as the model delta-function potentials on the same footing in the Kramers–Henneberger frame.

  2. Attosecond nonlinear optics using gigawatt-scale isolated attosecond pulses

    Science.gov (United States)

    Takahashi, Eiji J.; Lan, Pengfei; Mücke, Oliver D.; Nabekawa, Yasuo; Midorikawa, Katsumi

    2013-10-01

    High-energy isolated attosecond pulses required for the most intriguing nonlinear attosecond experiments as well as for attosecond-pump/attosecond-probe spectroscopy are still lacking at present. Here we propose and demonstrate a robust generation method of intense isolated attosecond pulses, which enable us to perform a nonlinear attosecond optics experiment. By combining a two-colour field synthesis and an energy-scaling method of high-order harmonic generation, the maximum pulse energy of the isolated attosecond pulse reaches as high as 1.3 μJ. The generated pulse with a duration of 500 as, as characterized by a nonlinear autocorrelation measurement, is the shortest and highest-energy pulse ever with the ability to induce nonlinear phenomena. The peak power of our tabletop light source reaches 2.6 GW, which even surpasses that of an extreme-ultraviolet free-electron laser.

  3. Attosecond nonlinear optics using gigawatt-scale isolated attosecond pulses.

    Science.gov (United States)

    Takahashi, Eiji J; Lan, Pengfei; Mücke, Oliver D; Nabekawa, Yasuo; Midorikawa, Katsumi

    2013-01-01

    High-energy isolated attosecond pulses required for the most intriguing nonlinear attosecond experiments as well as for attosecond-pump/attosecond-probe spectroscopy are still lacking at present. Here we propose and demonstrate a robust generation method of intense isolated attosecond pulses, which enable us to perform a nonlinear attosecond optics experiment. By combining a two-colour field synthesis and an energy-scaling method of high-order harmonic generation, the maximum pulse energy of the isolated attosecond pulse reaches as high as 1.3 μJ. The generated pulse with a duration of 500 as, as characterized by a nonlinear autocorrelation measurement, is the shortest and highest-energy pulse ever with the ability to induce nonlinear phenomena. The peak power of our tabletop light source reaches 2.6 GW, which even surpasses that of an extreme-ultraviolet free-electron laser.

  4. Attosecond electron pulse trains and quantum state reconstruction in ultrafast transmission electron microscopy

    Science.gov (United States)

    Priebe, Katharina E.; Rathje, Christopher; Yalunin, Sergey V.; Hohage, Thorsten; Feist, Armin; Schäfer, Sascha; Ropers, Claus

    2017-12-01

    Ultrafast electron and X-ray imaging and spectroscopy are the basis for an ongoing revolution in the understanding of dynamical atomic-scale processes in matter. The underlying technology relies heavily on laser science for the generation and characterization of ever shorter pulses. Recent findings suggest that ultrafast electron microscopy with attosecond-structured wavefunctions may be feasible. However, such future technologies call for means to both prepare and fully analyse the corresponding free-electron quantum states. Here, we introduce a framework for the preparation, coherent manipulation and characterization of free-electron quantum states, experimentally demonstrating attosecond electron pulse trains. Phase-locked optical fields coherently control the electron wavefunction along the beam direction. We establish a new variant of quantum state tomography—`SQUIRRELS'—for free-electron ensembles. The ability to tailor and quantitatively map electron quantum states will promote the nanoscale study of electron-matter entanglement and new forms of ultrafast electron microscopy down to the attosecond regime.

  5. Obtaining attosecond x-ray pulses using a self-amplified spontaneous emission free electron laser

    Directory of Open Access Journals (Sweden)

    A. A. Zholents

    2005-05-01

    Full Text Available We describe a technique for the generation of a solitary attosecond x-ray pulse in a free-electron laser (FEL, via a process of self-amplified spontaneous emission. In this method, electrons experience an energy modulation upon interacting with laser pulses having a duration of a few cycles within single-period wiggler magnets. Two consecutive modulation sections, followed by compression in a dispersive section, are used to obtain a single, subfemtosecond spike in the electron peak current. This region of the electron beam experiences an enhanced growth rate for FEL amplification. After propagation through a long undulator, this current spike emits a ∼250   attosecond x-ray pulse whose intensity dominates the x-ray emission from the rest of the electron bunch.

  6. Generation of isolated attosecond pulses with double optical gating and electronic dynamics in molecules studied via attosecond pump-probe experiment

    Science.gov (United States)

    Mashiko, Hiroki

    2010-03-01

    Single isolated attosecond pulses are useful tools for studying electron dynamics. Previously, such as pulses can be generated by few cycle 5 fs driving lasers. It is still a technical challenge to reproduce daily such pulses. In order to allow longer driving laser pulses, two optical gating methods of polarization gating and two-color gating are combined. This approach is dubbed double optical gating. Due to less depletion of the ground state population by the leading edge of the field, this technique can produce isolated 250 as pulses using up to ˜25 fs driving laser pulses. Also, the supercontinuous spectra (28-620 eV) can in principle support a 16 as pulse duration, obtained from 8 fs driving lasers. Because of the relaxation on the driving laser requirements, more laboratories can enter the isolated attosecond pulse science field. Pump-probe experiments with such isolated attosecond pulses and IR pulses can provide quantitative information on electronic dynamics. In recent work, the photoelectron spectra of sulfur hexafluoride (SF6) clearly indicates the precise shape of the IR driving pulse (1.5 eV), verifying that isolated ˜400 as pulses (93 eV) are achieved and these pulses produce an instantaneous inner valence ionization in the molecule. The pump-probe spectra of cation fragments resulting from double and triple ionization show 6-7 fs rise times (SF4^2+, SF3^2+, SF2^2+ and S^2+) or decay times (SF^+ and S^+) times governed by the overlap of the IR and XUV pulses. A suppression or enhancement of certain fragmentation channels is tentatively interpreted as resulting from the IR laser exciting the initial cations to higher states that exhibit different decay channels. This type of pump-probe experiment with isolated attosecond pulses is powerful for the study of electronic dynamics as well as resulting nuclear fragmentation measurements.

  7. Generating stable attosecond x-ray pulse trains with a mode-locked seeded free-electron laser

    Directory of Open Access Journals (Sweden)

    Chao Feng

    2012-08-01

    Full Text Available Generation of attosecond x-ray pulses is attracting much attention within the x-ray free-electron laser (FEL user community. We propose a novel scheme for the generation of coherent stable attosecond x-ray pulse trains in a seeded FEL, via a process of mode-locked amplification. Three modulators and two chicanes are used for generating separated attosecond scale microstructures in the electron beam using the beam echo effect. Such electron beam will produce high harmonic radiation with a comb of longitudinal modes at the very beginning of the radiator. By using a series of spatiotemporal shifts between the copropagating radiation and electron beam in the radiator, all these modes can be preserved and amplified to saturation. Using a representative realistic set of parameters, three-dimensional simulation results show that trains of 200 attosecond soft x-ray pulses with stable peak powers at gigawatt level can be generated directly from ultraviolet seed lasers. The even spacing between the attosecond pulses can be easily altered from subfemtosecond to tens of femtoseconds by slightly changing the wavelength of one seed laser.

  8. Circularly polarized attosecond pulse generation and applications to ultrafast magnetism

    Science.gov (United States)

    Bandrauk, André D.; Guo, Jing; Yuan, Kai-Jun

    2017-12-01

    Attosecond science is a growing new field of research and potential applications which relies on the development of attosecond light sources. Achievements in the generation and application of attosecond pulses enable to investigate electron dynamics in the nonlinear nonperturbative regime of laser-matter interactions on the electron’s natural time scale, the attosecond. In this review, we describe the generation of circularly polarized attosecond pulses and their applications to induce attosecond magnetic fields, new tools for ultrafast magnetism. Simulations are performed on aligned one-electron molecular ions by using nonperturbative nonlinear solutions of the time-dependent Schrödinger equation. We discuss how bichromatic circularly polarized laser pulses with co-rotating or counter-rotating components induce electron-parent ion recollisions, thus producing circularly polarized high-order harmonic generation, the source of circularly polarized attosecond pulses. Ultrafast quantum electron currents created by the generated attosecond pulses give rise to attosecond magnetic field pulses. The results provide a guiding principle for producing circularly polarized attosecond pulses and ultrafast magnetic fields in complex molecular systems for future research in ultrafast magneto-optics.

  9. Characterization and Application of Isolated Attosecond Pulses

    Science.gov (United States)

    Wei, Hui

    Isolated attosecond pulse (IAP) is a tool of probing electronic dynamics occurring in atoms, molecules, clusters and solids, since the time scale of electronic motion is on the order of attoseconds. The generation, characterization and applications of IAPs has become one of the fast frontiers of laser experiments. This dissertation focuses on several aspects of attosecond physics. First, we study the driving wavelength scaling of the yield of high-order harmonic generation (HHG) by applying the quantum orbit theory. The unfavorable scaling law especially for the short quantum orbit is of great importance to attoseond pulse generation toward hundreds of eVs or keV photon energy region by mid-infrared (mid-IR) lasers. Second, we investigate the accuracy of the current frequency-resolved optical gating for complete reconstruction of attosecond bursts (FROG-CRAB) and phase retrieval by omega oscillation filtering (PROOF) methods for IAP characterization by simulating the experimental data by theoretical calculation. This calibration is critical but has not been carefully carried out before. We also present an improved method, namely the swPROOF which is more universal and robust than the original PROOF method. Third, we investigate the controversial topic of photoionization time delay. We find the limitation of the FROG-CRAB method which has been used to extract the photoionization time delay between the 2s and 2p channels in neon. The time delay retrieval is sensitive to the attochirp of the XUV pulse, which may lead to discrepancies between experiment and theory. A new fitting method is proposed in order to overcome the limitations of FROG-CRAB. Finally, IAPs are used to probe the dynamic of electron correlation in helium atom by means of attosecond transient absorption spectroscopy. The agreement between the measurement and our analytical model verifies the observation of time-dependent build up of the 2s2p Fano resonance.

  10. Measurement and Control of Attosecond Pulses

    Science.gov (United States)

    2016-04-25

    the re-collision electron wave packet and therefore on the attosecond pulse that it produces. This modification deflects the beam and the deflection ...TYPE. State the type of report, such as final, technical, interim, memorandum, master’s thesis , progress, quarterly, research, special, group study...illustrated in Figure 1. A weak beam is incident on the nonlinear medium at a slight angle to the fundamental. It imposes a phased modification on

  11. Nonlinear coherent Thomson scattering from relativistic electron sheets as a means to produce isolated ultrabright attosecond x-ray pulses

    Directory of Open Access Journals (Sweden)

    H.-C. Wu (武慧春

    2011-07-01

    Full Text Available A new way to generate intense attosecond x-ray pulses is discussed. It relies on coherent Thomson scattering (CTS from relativistic electron sheets. A double layer technique is used to generate planar solid-density sheets of monochromatic high-γ electrons with zero transverse momentum such that coherently backscattered light is frequency upshifted by factors up to 4γ^{2}. Here previous work [H.-C. Wu et al., Phys. Rev. Lett. 104, 234801 (2010PRLTAO0031-900710.1103/PhysRevLett.104.234801] is extended to the regime of high-intensity probe light with normalized amplitude a_{0}>1 leading to nonlinear CTS effects such as pulse contraction and steepening. The results are derived both by particle-in-cell (PIC simulation in a boosted frame and by analytic theory. PIC simulation shows that powerful x-ray pulses (1 keV, 10   gigawatt can be generated. They call for experimental verification. Required prerequisites such as manufacture of nanometer-thick target foils is ready and ultrahigh contrast laser pulses should be within reach in the near future.

  12. Imaging attosecond electron wavepackets around the ionization threshold

    Energy Technology Data Exchange (ETDEWEB)

    Swoboda, Marko; Remetter, Thomas; Mauritsson, Johan; L' Huillier, Anne [Dept. of Physics, Lund University (Sweden); Schafer, Kenneth J. [Louisiana State Univ., Baton Rouge, Louisiana (United States); Kelkensberg, Freek; Siu, Wing-Kiu; Johnsson, Per; Vrakking, Marc J.J. [AMOLF Institute, Amsterdam (Netherlands); Kling, Matthias F.; Znakovskaya, Irina; Uphues, Thorsten; Zherebtsov, Sergey [MPI fuer Quantenoptik, Garching (Germany); Lepine, Franck [Univ. Lyon 1, CNRS, LASIM, UMR, Villeurbanne (France); Benedetti, Enrico; Ferrari, Federico; Sansone, Giuseppe; Nisoli, Mauro [CUSBO, ULTRAS-INFM, Politecnico, Milano (Italy)

    2008-07-01

    We image the momentum distributions of attosecond electron wavepackets generated from the ionization of Helium by attosecond XUV pulses. Using an infrared probing field, the evolution of these wavepackets can be captured in time and space. Tuning the central frequency of the pulses allows us to initiate a number of processes that originate from the interplay of partially bound and continuum wavepackets or returning electrons and the atomic potential. Using this attosecond pump-probe scheme, we can track electron dynamics around the ionization barrier, performing interferometric measurements of different ionization pathways.

  13. Attosecond pump-probe electron interferometry

    CERN Document Server

    Mauritsson, J; Swoboda, M; Klunder, K; L'Huillier, A; Schafer, K J; Ghafur, O; Kelkensberg, F; Siu, W; Johnsson, P; Vrakking, M J J; Znakovskaya, I; Uphues, T; Zherebtsov, S; Kling, M F; Lepine, F; Benedetti, E; Ferrari, F; Sansone, G; Nisoli, M

    2010-01-01

    Attosecond science has as its goal the measurement and ultimately the control of electron dynamics on its natural time scale, the atomic unit of time, which is 24 attoseconds. The short pulses required to reach this time scale imply large bandwidths, leading to the excitation not of a single state but of a broad and coherent superposition of states, i.e., a wave packet. In this paper we present a novel interferometric method that uses a free wave packet as a reference to measure a bound wave packet. The resulting interferogram contains both quantum beats as well as multi-path interference and provides precise and state-specific time-resolved amplitude and phase information about the bound electron wave packet. We demonstrate our method experimentally by measuring a bound attosecond wave packet in helium, prepared using an isolated 350 attosecond pulse with a central energy in the vicinity of the ionization threshold. In addition we show that our approach can also be applied to bound wave packets irrespective ...

  14. Nano-plasmonic near field phase matching of attosecond pulses.

    Science.gov (United States)

    Shaaran, Tahir; Nicolas, Rana; Iwan, Bianca; Kovacev, Milutin; Merdji, Hamed

    2017-07-25

    Nano-structures excited by light can enhance locally the electric field when tuned to plasmonic resonances. This phenomenon can be used to boost non-linear processes such as harmonic generation in crystals or in gases, Raman excitation, and four wave mixing. Here we present a theoretical investigation of the near-field phase matching of attosecond pulses emitted by high-order harmonic generation (HHG) of an atom immersed in a multi-cycle femtosecond infrared laser field and a spatially inhomogeneous plasmonic field. We demonstrate that the spatial inhomogeneity factor of the plasmonic field strongly affects the electron trajectory and recombination time which can be used to control the attosecond emission. For further insight into the plasmonic field effect, we monitor the phase of each quantum path as a function of the inhomogeneity strength. Moreover, we investigate the attosecond emission as a function of near-field phase matching effects. This is achieved by calculating the coherent field superposition of attosecond pulses emitted from various intensities or field inhomogeneities. Finally, far-field and near-field phase matching effects are combined to modulate the harmonic spectral phase towards the emission of a single attosecond pulse.

  15. Macroscopic effects in attosecond pulse generation

    Energy Technology Data Exchange (ETDEWEB)

    Ruchon, T; Varju, K; Mansten, E; Swoboda, M; L' Huillier, A [Department of Physics, Lund University, PO Box 118, SE-221 00 Lund (Sweden); Hauri, C P; Lopez-Martens, R [Laboratoire d' Optique Appliquee, Ecole Nationale Superieure des Techniques Avancees (ENSTA)-Ecole Polytechnique CNRS UMR 7639, 91761 Palaiseau (France)], E-mail: anne.lhuillier@fysik.lth.se

    2008-02-15

    We examine how the generation and propagation of high-order harmonics in a partly ionized gas medium affect their strength and synchronization. The temporal properties of the resulting attosecond pulses generated in long gas targets can be significantly influenced by macroscopic effects, in particular by the intensity in the medium and the degree of ionization which control the dispersion. Under some conditions, the use of gas targets longer than the absorption length can lead to the generation of compressed attosecond pulses. We show these macroscopic effects experimentally, using a 6 mm-long argon-filled gas cell as the generating medium.

  16. Single 100-terawatt attosecond X-ray light pulse generation

    CERN Document Server

    Xu, X R; Zhang, Y X; Lu, H Y; Zhang, H; Dromey, B; Zhu, S P; Zhou, C T; Zepf, M; He, X T

    2016-01-01

    The birth of attosecond light sources is expected to inspire a breakthrough in ultrafast optics, which may extend human real-time measurement and control techniques into atomic-scale electronic dynamics. For applications, it is essential to obtain a single attosecond pulse of high intensity, large photon energy and short duration. Here we show that single 100-terawatt attosecond X-ray light pulse with intensity ${1\\times10^{21}}\\textrm{W}/\\textrm{cm}^{{ 2}}$ and duration ${7.9} \\textrm{as}$ can be produced by intense laser irradiation on a capacitor-nanofoil target composed of two separate nanofoils. In the interaction, a strong electrostatic potential develops between two nanofoils, which drags electrons out of the second foil and piles them up in vacuum, forming an ultradense relativistic electron nanobunch. This nanobunch exists in only half a laser cycle and smears out in others, resulting in coherent synchrotron emission of a single pulse. Such an unprecedentedly giant attosecond X-ray pulse may bring us...

  17. Obtaining two attosecond pulses pulses for x-ray stimulated Raman spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Zholents, Alexander; Penn, G.

    2009-06-23

    Attosecond x-ray pulses are an indispensable tool for the study of electronic and structural changes in molecules undergoing chemical reactions. They have a wide bandwidth comparable to the energy bands of valence electronic states and, therefore, are well suited for making and probing multiple valence electronic excitations using core electron transitions. Here we propose a method of creating a sequence of two attosecond soft x-ray pulses in a free electron laser by optical manipulation of electrons located in two different sections of the electron bunch. The energy of each x-ray pulse can be of the order of 100 nJ and the pulse width of the order of 250 attoseconds. The carrier frequency of each x-ray pulse can be independently tuned to a resonant core electron transition of a specific atom of the molecule. The time interval between the two attosecond pulses is tunable from a few femtoseconds to a hundred femtoseconds with better than 100 attoseconds precision.

  18. Attomicroscopy: from femtosecond to attosecond electron microscopy

    Science.gov (United States)

    Hassan, Mohammed Th

    2018-02-01

    In the last decade, the development of ultrafast electron diffraction (UED) and microscopy (UEM) have enabled the imaging of atomic motion in real time and space. These pivotal table-top tools opened the door for a vast range of applications in different areas of science spanning chemistry, physics, materials science, and biology. We first discuss the basic principles and recent advancements, including some of the important applications, of both UED and UEM. Then, we discuss the recent advances in the field that have enhanced the spatial and temporal resolutions, where the latter, is however, still limited to a few hundreds of femtoseconds, preventing the imaging of ultrafast dynamics of matter lasting few tens of femtoseconds. Then, we present our new optical gating approach for generating an isolated 30 fs electron pulse with sufficient intensity to attain a temporal resolution on the same time scale. This achievement allows, for the first time, imaging the electron dynamics of matter. Finally, we demonstrate the feasibility of the optical gating approach to generate an isolated attosecond electron pulse, utilizing our recently demonstrated optical attosecond laser pulse, which paves the way for establishing the field of ‘Attomicroscopy’, ultimately enabling us to image the electron motion in action.

  19. Self-amplified spontaneous emission FEL with energy-chirped electron beam and its application for generation of attosecond x-ray pulses

    Directory of Open Access Journals (Sweden)

    E. L. Saldin

    2006-05-01

    Full Text Available Influence of a linear energy chirp in the electron beam on a self-amplified spontaneous emission (SASE Free Electron Laser (FEL operation is studied analytically and numerically using a 1D model. Analytical results are based on the theoretical background developed by Krinsky and Huang [Phys. Rev. ST Accel. Beams 6, 050702 (2003PRABFM1098-4402]. Explicit expressions for Green’s functions and for output power of a SASE FEL are obtained for the high-gain linear regime in the limits of small and large energy chirp parameters. Saturation length and power versus energy chirp parameter are calculated numerically. It is shown that the effect of linear energy chirp on FEL gain is equivalent to the linear undulator tapering (or linear energy variation along the undulator. A consequence of this fact is a possibility to perfectly compensate FEL gain degradation, caused by the energy chirp, by means of the undulator tapering independently of the value of the energy chirp parameter. An application of this effect for generation of attosecond pulses from a hard x-ray FEL is proposed. Strong energy modulation within a short slice of an electron bunch is produced by a few-cycle optical laser pulse in a short undulator, placed in front of the main undulator. Gain degradation within this slice is compensated by an appropriate undulator taper while the rest of the bunch suffers from this taper and does not lase. Three-dimensional simulations predict that short (200 attoseconds high-power (up to 100 GW pulses can be produced in Angstrom wavelength range with a high degree of contrast. A possibility to reduce pulse duration to sub-100 attosecond scale is discussed.

  20. Attosecond photoelectron spectroscopy of electron transport in solids

    Energy Technology Data Exchange (ETDEWEB)

    Magerl, Elisabeth

    2011-03-31

    Time-resolved photoelectron spectroscopy of condensed matter systems in the attosecond regime promises new insights into excitation mechanisms and transient dynamics of electrons in solids. This timescale became accessible directly only recently with the development of the attosecond streak camera and of laser systems providing few-cycle, phase-controlled laser pulses in the near-infrared, which are used to generate isolated, sub-femtosecond extreme-ultraviolet pulses with a well-defined timing with respect to the near-infrared pulse. Employing these pulses, the attosecond streak camera offers time resolutions as short as a few 10 attoseconds. In the framework of this thesis, a new, versatile experimental apparatus combining attosecond pulse generation in gases with state of the art surface science techniques is designed, constructed, and commissioned. Employing this novel infrastructure and the technique of the attosecond transient recorder, we investigate transport phenomena occurring after photoexcitation of electrons in tungsten and rhenium single crystals and show that attosecond streaking is a unique method for resolving extremely fast electronic phenomena in solids. It is demonstrated that electrons originating from different energy levels, i.e. from the conduction band and the 4f core level, are emitted from the crystal surface at different times. The origin of this time delay, which is below 150 attoseconds for all studied systems, is investigated by a systematic variation of several experimental parameters, in particular the photon energy of the employed attosecond pulses. These experimental studies are complemented by theoretical studies of the group velocity of highly-excited electrons based on ab initio calculations. While the streaking technique applied on single crystals can provide only information about the relative time delay between two types of photoelectrons, the absolute transport time remains inaccessible. We introduce a scheme of a reference

  1. Electron Interference in Molecular Circular Polarization Attosecond XUV Photoionization

    Directory of Open Access Journals (Sweden)

    Kai-Jun Yuan

    2015-01-01

    Full Text Available Two-center electron interference in molecular attosecond photoionization processes is investigated from numerical solutions of time-dependent Schrödinger equations. Both symmetric H\\(_2^+\\ and nonsymmetric HHe\\(^{2+}\\ one electron diatomic systems are ionized by intense attosecond circularly polarized XUV laser pulses. Photoionization of these molecular ions shows signature of interference with double peaks (minima in molecular attosecond photoelectron energy spectra (MAPES at critical angles \\(\\vartheta_c\\ between the molecular \\(\\textbf{R}\\ axis and the photoelectron momentum \\(\\textbf{p}\\. The interferences are shown to be a function of the symmetry of electronic states and the interference patterns are sensitive to the molecular orientation and pulse polarization. Such sensitivity offers possibility for imaging of molecular structure and orbitals.

  2. Generation and Characterization of Attosecond Pulses

    Energy Technology Data Exchange (ETDEWEB)

    Ian A. Walmsley; Robert W. Boyd

    2006-04-24

    The research undertaken in this project has been directed toward the area of attoscience, in particular the problem of attosecond metrology. That is, the accurate determination of the electric field of attosecond XUV radiation. This outstanding problem has been identified as a critical technology for further development of the field, and our research adds to the area by providing the first method for characterization using the harmonic radiation itself as a tool. The technical effectiveness of this approach is very high, since it is vastly easier to detect XUV radiation directly than via the spectrum of photoelectrons liberated from atoms by it. This means that the experimental data rate can be much higher in principle using all-optical detection that electron detection, which will greatly aid the utility of harmonic XUV sources in attoscience applications. There are as yet no direct public benefits from this area of scientific research, though access to material structural dynamics on unprecedented brief timescales are expected to yield significant benefits for the future.

  3. Producing High Intense Attosecond Pulse Train by Interaction of Three-Color Pulse and Overdense Plasma

    Science.gov (United States)

    Salehi, M.; Mirzanejad, S.

    2017-05-01

    Amplifying the attosecond pulse by the chirp pulse amplification method is impossible. Furthermore, the intensity of attosecond pulse is low in the interaction of laser pulse and underdense plasma. This motivates us to propose using a multi-color pulse to produce the high intense attosecond pulse. In the present study, the relativistic interaction of a three-color linearly-polarized laser-pulse with highly overdense plasma is studied. We show that the combination of {{ω }}1, {{ω }}2 and {{ω }}3 frequencies decreases the instance full width at half maximum reflected attosecond pulse train from the overdense plasma surface. Moreover, we show that the three-color pulse increases the intensity of generated harmonics, which is explained by the relativistic oscillating mirror model. The obtained results demonstrate that if the three-color laser pulse interacts with overdense plasma, it will enhance two orders of magnitude of intensity of ultra short attosecond pulses in comparison with monochromatic pulse.

  4. Generation of isolated single attosecond hard X-ray pulse in enhanced self-amplified spontaneous emission scheme.

    Science.gov (United States)

    Kumar, Sandeep; Kang, Heung-Sik; Kim, Dong Eon

    2011-04-11

    The generation of isolated attosecond hard x-ray pulse has been studied under the enhanced self-amplified spontaneous emission (ESASE) scheme with the density and energy modulation of an electron bunch. It is demonstrated in simulation that an isolated attosecond hard x-ray pulse of a high contrast ratio can be produced by adjusting a driver laser wavelength and the energy distribution of an electron bunch. An isolated attosecond pulse of ~146 attosecond full-width half-maximum (FWHM) at 0.1 nm wavelength is obtained with a saturation length of 34 meter for the electron beam parameters of Korean X-ray Free Electron laser. © 2011 Optical Society of America

  5. Probing attosecond pulse structures by XUV-induced hole dynamics

    CERN Document Server

    You, Jhih-An; Dahlström, Jan Marcus

    2015-01-01

    We investigate a two-photon ionization process in neon by an isolated attosecond pump pulse and two coherent extreme ultraviolet probe fields. The probe fields, tuned to the 2s-2p transition in the residual ion, allow for coherent control of the photoelectron via indirect interactions with the hole. We show that the photoelectron-ion coincidence signal contains an interference pattern that can be used to reconstruct the temporal structure of attosecond pump pulses. Our results are supported by simulations based on time-dependent configuration-interaction singles and lowest-order perturbation theory within second quantization.

  6. Harmonic and attosecond pulse enhancement in the presence of noise

    Science.gov (United States)

    Feng, Li-Qiang; Chu, Tian-Shu

    2012-12-01

    In this paper, we theoretically investigate the effect of noise on the photoionization, the generation of the high-order harmonic and the attosecond pulse irradiated from a model He+ ion. It shows that by properly adding noise fields, such as Gaussian white noise, random light or colored noise, both the ionization probabilities (IPs) and the harmonic yields can be enhanced by several orders of magnitude. Further, by tuning the noise intensity, a stochastic resonance-like curve is observed, showing the existence of an optimal noise in the ionization enhancement process. Finally, by superposing a properly selected harmonic, an intense attosecond pulse with a duration of 67 as is directly generated.

  7. Single attosecond pulse production with an ellipticity-modulated driving IR pulse

    Energy Technology Data Exchange (ETDEWEB)

    Strelkov, V [CELIA, Universite Bordeaux 1, 351 Cours de la liberation, 33405 Talence (France); Zair, A [CELIA, Universite Bordeaux 1, 351 Cours de la liberation, 33405 Talence (France); Tcherbakoff, O [CELIA, Universite Bordeaux 1, 351 Cours de la liberation, 33405 Talence (France); Lopez-Martens, R [Department of Physics, Lund Institute of Technology, PO Box 118, S-22100, Lund (Sweden); Cormier, E [CELIA, Universite Bordeaux 1, 351 Cours de la liberation, 33405 Talence (France); Mevel, E [CELIA, Universite Bordeaux 1, 351 Cours de la liberation, 33405 Talence (France); Constant, E [CELIA, Universite Bordeaux 1, 351 Cours de la liberation, 33405 Talence (France)

    2005-05-28

    We theoretically study attosecond pulse production via high-harmonic generation using a driving laser pulse with a time-dependent ellipticity. The theoretical approach produces results that agree with our experimental data obtained using 35 fs driving laser pulses and is further used to study the generation of single attosecond pulses with shorter laser pulses. We find an equation for the duration of the temporal window created by the time-varying driving laser polarization in which high-harmonic emission can occur. We formulate the necessary requirements concerning the driving laser field in order to confine the high-harmonic emission in the form of a single attosecond pulse. Indeed, we show that using incident 12 fs laser pulses single attosecond pulses can be produced for certain carrier-envelope phase (CEP) values of the driving pulse. For 6 fs incident laser pulses, single attosecond pulses are produced for all values of the CEP (the intensity of the attosecond pulse still depends on the actual value of the CEP). If implemented with state-of-the-art 5 fs laser pulses, this technique can even lead to the production of sub-100 as pulses. (letter to the editor)

  8. Attosecond Control of Photoabsorption Through Manipulating the Electron-Electron Correlation

    Science.gov (United States)

    Hu, S. X.

    2014-05-01

    This talk reports on studies of photoabsorption control by manipulating the electron -electron correlation in a double-ionization process with an attosecond extreme ultraviolet (EUV) pulse. Electron correlation plays an essential role in a wide range of fundamentally important many-body phenomena in modern physics and chemistry. An example is the importance of electron-electron correlation in multiple ionization of multielectron atoms and molecules exposed to intense laser pulses. Manipulating the dynamic electron correlation in such photoinduced processes is a crucial step toward the coherent control of chemical reactions and photobiological processes. We will show for the first time, from full-dimensional ab initio calculations of double ionization of helium in intense laser pulses (λ = 780 nm), that the electron-electron interactions can be instantaneously tuned using a time-delayed attosecond EUV pulse. Consequently, the probability of producing energetic electrons from excessive photoabsorption can be enhanced by an order of magnitude through the attosecond control of electron-electron correlation. This work was partially supported by the Department of Energy National Nuclear Security Administration under Award No. DE-NA0001944, the University of Rochester, and the New York State Energy Research and Development Authority. Computations have been conducted utilizing the ``Kraken'' Supercomputer at NICS.

  9. High-throughput beamline for attosecond pulses based on toroidal mirrors with microfocusing capabilities.

    Science.gov (United States)

    Frassetto, F; Trabattoni, A; Anumula, S; Sansone, G; Calegari, F; Nisoli, M; Poletto, L

    2014-10-01

    We have developed a novel attosecond beamline designed for attosecond-pump/attosecond probe experiments. Microfocusing of the Extreme-ultraviolet (XUV) radiation is obtained by using a coma-compensated optical configuration based on the use of three toroidal mirrors controlled by a genetic algorithm. Trains of attosecond pulses are generated with a measured peak intensity of about 3 × 10(11) W/cm(2).

  10. Attosecond pulse characterization with coherent Rydberg wavepackets

    CERN Document Server

    Pabst, Stefan

    2016-01-01

    We propose a new technique to fully characterize the temporal structure of extreme ultraviolet pulses by ionizing a bound coherent electronic wavepacket. The populated energy levels make it possible to interfere different spectral components leading to quantum beats in the photoelectron spectrum as a function of the delay between ionization and initiation of the wavepacket. The influence of the dipole phase, which is the main obstacle for state-of-the-art pulse characterization schemes, can be eliminated by angle integration of the photoelectron spectrum. We show that particularly atomic Rydberg wavepackets are ideal and that wavepackets involving multiple electronic states provide redundant information which can be used to cross-check the consistency of the phase reconstruction.

  11. Optical circular deflector with attosecond resolution for ultrashort electron beam

    Directory of Open Access Journals (Sweden)

    Zhen Zhang

    2017-05-01

    Full Text Available A novel method using high-power laser as a circular deflector is proposed for the measurement of femtosecond (fs and sub-fs electron beam. In the scheme, the electron beam interacts with a laser pulse operating in a radially polarized doughnut mode (TEM_{01^{*}} in a helical undulator, generating angular kicks along the beam in two directions at the same time. The phase difference between the two angular kicks makes the beam form a ring after a propagation section with appropriate phase advance, which can reveal the current profile of the electron beam. Detailed theoretical analysis of the method and numerical results with reasonable parameters are both presented. It is shown that the temporal resolution can reach up to ∼100 attosecond, which is a significant improvement for the diagnostics of ultrashort electron beam.

  12. Generation of attosecond soft X-ray pulses in a longitudinal space charge amplifier

    Energy Technology Data Exchange (ETDEWEB)

    Dohlus, M.; Schneidmiller, E.A.; Yurkov, M.V. [Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)

    2011-03-15

    A longitudinal space charge amplifier (LSCA), operating in soft X-ray regime, was recently proposed. Such an amplifier consists of a few amplification cascades (focusing channel and chicane) and a short radiator undulator in the end. Broadband nature of LSCA supports generation of few-cycle pulses as well as wavelength compression. In this paper we consider an application of these properties of LSCA for generation of attosecond X-ray pulses. It is shown that a compact and cheap addition to the soft X-ray free electron laser facility FLASH would allow to generate 60 attosecond (FWHM) long X-ray pulses with the peak power at 100 MW level and a contrast above 98%. (orig.)

  13. Spectral shaping of attosecond pulses using two-colour laser fields

    Energy Technology Data Exchange (ETDEWEB)

    Mansten, E; Dahlstroem, J M; Johnsson, P; Swoboda, M; L' Huillier, A; Mauritsson, J [Department of Physics, Lund University, P O Box 118, SE-221 00 Lund (Sweden)], E-mail: erik.mansten@fysik.lth.se, E-mail: johan.mauritsson@fysik.lth.se

    2008-08-15

    We use a strong two-colour laser field composed of the fundamental (800 nm) and the second harmonic (400 nm) of an infrared (IR) laser field to generate attosecond pulses with controlled spectral and temporal properties. With a second-harmonic intensity equal to 15% of the IR intensity the second-harmonic field is strong enough to significantly alter and control the electron trajectories in the generation process. This enables us to tune the central photon energy of the attosecond pulses by changing the phase difference between the IR and the second-harmonic fields. In the time domain the radiation is emitted as a sequence of pulses separated by a full IR cycle. We also perform calculations showing that the effect of even stronger second-harmonic fields leads to an extended tunable range under conditions that are experimentally feasible.

  14. Spectral enhancement of single attosecond pulses by time-delayed control field

    CERN Document Server

    Chu, Wei-Chun

    2012-01-01

    An optical coherent control scheme has been proposed where an extreme ultraviolet single attosecond pulse (SAP) propagates through a dense helium gas dressed by a time-delayed femtosecond laser pulse. The laser pulse couples the 2s2p(^1P) and 2s^2(^1S) autoionizing states when the SAP excites the 2s2p state. After going through the gas, the spectral and temporal profiles of the SAP are strongly distorted. A narrowed but enhanced spike in the spectrum shows up for specific intensities and time delays of the laser, which exemplifies the control of a broadband photon wave packet by an ultrashort dressing field for the first time. We analyze the photon and electron dynamics and conclude on the dressing condition that maximizes this enhancement. The result demonstrates new possibilities of attosecond optical control.

  15. Coherent hard x rays from attosecond pulse train-assisted harmonic generation.

    Science.gov (United States)

    Klaiber, Michael; Hatsagortsyan, Karen Z; Müller, Carsten; Keitel, Christoph H

    2008-02-15

    High-order harmonic generation from atomic systems is considered in the crossed fields of a relativistically strong infrared laser and a weak attosecond pulse train of soft x rays. Due to one-photon ionization by the x-ray pulse, the ionized electron obtains a starting momentum that compensates the relativistic drift, which is induced by the laser magnetic field, and allows the electron to efficiently emit harmonic radiation upon recombination with the atomic core in the relativistic regime. This way, short pulses of coherent hard x rays of up to 40 keV energy can be generated.

  16. Generation of attosecond electron bunches in a laser-plasma accelerator using a plasma density upramp

    Energy Technology Data Exchange (ETDEWEB)

    Weikum, M.K., E-mail: maria.weikum@desy.de [Deutsches Elektronensynchrotron (DESY), Bdg. 30b, Notkestr. 85, 22607 Hamburg (Germany); Department of Physics, University of Strathclyde, G4 0NG Glasgow (United Kingdom); Li, F.Y. [Department of Physics, University of Strathclyde, G4 0NG Glasgow (United Kingdom); Assmann, R.W. [Deutsches Elektronensynchrotron (DESY), Bdg. 30b, Notkestr. 85, 22607 Hamburg (Germany); Sheng, Z.M. [Department of Physics, University of Strathclyde, G4 0NG Glasgow (United Kingdom); Laboratory for Laser Plasmas and Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Jaroszynski, D. [Department of Physics, University of Strathclyde, G4 0NG Glasgow (United Kingdom)

    2016-09-01

    Attosecond electron bunches and attosecond radiation pulses enable the study of ultrafast dynamics of matter in an unprecedented regime. In this paper, the suitability for the experimental realization of a novel scheme producing sub-femtosecond duration electron bunches from laser-wakefield acceleration in plasma with self-injection in a plasma upramp profile has been investigated. While it has previously been predicted that this requires laser power above a few hundred terawatts typically, here we show that the scheme can be extended with reduced driving laser powers down to tens of terawatts, generating accelerated electron pulses with minimum length of around 166 attoseconds and picocoulombs charge. Using particle-in-cell simulations and theoretical models, the evolution of the accelerated electron bunch within the plasma as well as simple scalings of the bunch properties with initial laser and plasma parameters are presented. - Highlights: • LWFA with an upramp density profile can trap and accelerate sub-fs electron beams. • A reduction of the necessary threshold laser intensity by a factor 4 is presented. • Electron properties are tuned by varying initial laser and plasma parameters. • Simulations predict electron bunch lengths below 200 attoseconds with pC charge. • Strong bunch evolution effects and a large energy spread still need to be improved.

  17. Coherent hard x-rays from attosecond pulse train-assisted harmonic generation

    OpenAIRE

    Klaiber, Michael; Hatsagortsyan, Karen Z.; Müller, Carsten; Keitel, Christoph H.

    2007-01-01

    High-order harmonic generation from atomic systems is considered in the crossed fields of a relativistically strong infrared laser and a weak attosecond-pulse train of soft x-rays. Due to one-photon ionization by the x-ray pulse, the ionized electron obtains a starting momentum that compensates the relativistic drift which is induced by the laser magnetic field, and allows the electron to efficiently emit harmonic radiation upon recombination with the atomic core in the relativistic regime. I...

  18. Attosecond control of orbital parity mix interferences and the relative phase of even and odd harmonics in an attosecond pulse train.

    Science.gov (United States)

    Laurent, G; Cao, W; Li, H; Wang, Z; Ben-Itzhak, I; Cocke, C L

    2012-08-24

    We experimentally demonstrate that atomic orbital parity mix interferences can be temporally controlled on an attosecond time scale. Electron wave packets are formed by ionizing argon gas with a comb of odd and even high-order harmonics, in the presence of a weak infrared field. Consequently, a mix of energy-degenerate even and odd parity states is fed in the continuum by one- and two-photon transitions. These interfere, leading to an asymmetric electron emission along the polarization vector. The direction of the emission can be controlled by varying the time delay between the comb and infrared field pulses. We show that such asymmetric emission provides information on the relative phase of consecutive odd and even order harmonics in the attosecond pulse train.

  19. Secondary-electron cascade in attosecond photoelectron spectroscopy from metals

    DEFF Research Database (Denmark)

    Baggesen, Jan Conrad; Madsen, Lars Bojer

    2009-01-01

    Attosecond spectroscopy is currently restricted to photon energies around 100 eV. We show that under these conditions, electron-electron scatterings, as the photoelectrons leave the metal, give rise to a tail of secondary electrons with lower energies and hence a significant background. We develop...

  20. Generation of Attosecond Light Pulses from Gas and Solid State Media

    Directory of Open Access Journals (Sweden)

    Stefanos Chatziathanasiou

    2017-03-01

    Full Text Available Real-time observation of ultrafast dynamics in the microcosm is a fundamental approach for understanding the internal evolution of physical, chemical and biological systems. Tools for tracing such dynamics are flashes of light with duration comparable to or shorter than the characteristic evolution times of the system under investigation. While femtosecond (fs pulses are successfully used to investigate vibrational dynamics in molecular systems, real time observation of electron motion in all states of matter requires temporal resolution in the attosecond (1 attosecond (asec = 10−18 s time scale. During the last decades, continuous efforts in ultra-short pulse engineering led to the development of table-top sources which can produce asec pulses. These pulses have been synthesized by using broadband coherent radiation in the extreme ultraviolet (XUV spectral region generated by the interaction of matter with intense fs pulses. Here, we will review asec pulses generated by the interaction of gas phase media and solid surfaces with intense fs IR laser fields. After a brief overview of the fundamental process underlying the XUV emission form these media, we will review the current technology, specifications and the ongoing developments of such asec sources.

  1. Generating ultrarelativistic attosecond electron bunches with laser wakefield accelerators

    NARCIS (Netherlands)

    Luttikhof, M.J.H.; Khachatryan, A.G.; van Goor, F.A.; Boller, Klaus J.

    2010-01-01

    Femtosecond electron bunches with ultrarelativistic energies were recently generated by laser wakefield accelerators. Here we predict that laser wakefield acceleration can generate even attosecond bunches, due to a strong chirp of the betatron frequency. We show how the bunch duration scales with

  2. Attosecond gamma-ray pulses via nonlinear Compton scattering in the radiation dominated regime

    CERN Document Server

    Li, Jian-Xing; Galow, Benjamin J; Keitel, Christoph H

    2015-01-01

    The interaction of a relativistic electron bunch with a counter-propagating tightly-focused laser beam is investigated for intensities when the dynamics is strongly affected by its own radiation. The Compton scattering spectra of gamma-radiation are evaluated employing a semiclassical description for the laser-driven electron dynamics and a quantum electrodynamical description for the photon emissions. We show for laser facilities under construction that gamma-ray bursts of few hundred attoseconds and dozens of megaelectronvolt photon energies may be detected in the near-backwards direction of the initial electron motion. Tight focussing of the laser beam and radiation reaction are demonstrated to be jointly responsible for such short gamma-ray bursts which are independent of both duration of electron bunch and laser pulse. Furthermore, the stochastic nature of the gamma-photon emission features signatures in the resulting gamma-ray comb in the case of the application of a multi-cycle laser pulse.

  3. Probing electronic binding potentials with attosecond photoelectron wavepackets

    Science.gov (United States)

    Kiesewetter, D.; Jones, R. R.; Camper, A.; Schoun, S. B.; Agostini, P.; Dimauro, L. F.

    2018-01-01

    The central goal of attosecond science is to visualize, understand and ultimately control electron dynamics in matter over the fastest relevant timescales. To date, numerous schemes have demonstrated exquisite temporal resolution, on the order of ten attoseconds, in measurements of the response of photo-excited electrons to time-delayed probes. However, attributing this response to specific dynamical mechanisms is difficult, requiring guidance from advanced calculations. Here we show that energy transfer between an oscillating field and low-energy attosecond photoelectron wavepackets directly provides coarse-grained information on the effective binding potential from which the electrons are liberated. We employ a dense extreme ultraviolet (XUV) harmonic comb to photoionize He, Ne and Ar atoms and record the electron spectra as a function of the phase of a mid-infrared dressing field. The amplitude and phase of the resulting interference modulations in the electron spectra reveal the average momentum and change in momentum of the electron wavepackets during the first quarter-period of the dressing field after their creation, reflecting the corresponding coarse characteristics of the binding potential.

  4. Generation of isolated attosecond pulses by spatial shaping of a femtosecond laser beam

    Energy Technology Data Exchange (ETDEWEB)

    Strelkov, V V; Mevel, E; Constant, E [Centre Lasers Intenses et Applications (CELIA), Domaine du Haut-Carre, Universite Bordeaux 1, 43 Rue Pierre Noailles, 33405 Talence (France)], E-mail: v-strelkov@fpl.gpi.ru

    2008-08-15

    We present a new method for generating isolated attosecond pulses via high-order harmonic generation in gases. It relies on using collective effects to achieve transient phase-matching which provides both a high efficiency and a strong temporal confinement under specific conditions. By controlling the spatial shape of the fundamental beam and the geometry of the laser-gas interaction, this transient phase matching leads to the generation of isolated broadband attosecond pulses with long driving pulses (10-20 fs) even without controlling their carrier envelope phase. Such laser pulses are becoming available at high energy levels and our approach offers a route to increase the energy of isolated attosecond pulses by orders of magnitude as compared to existing sources.

  5. Distinguishing attosecond electron-electron scattering and screening in transition metals

    Science.gov (United States)

    Chen, Cong; Tao, Zhensheng; Carr, Adra; Matyba, Piotr; Szilvási, Tibor; Emmerich, Sebastian; Piecuch, Martin; Keller, Mark; Zusin, Dmitriy; Eich, Steffen; Rollinger, Markus; You, Wenjing; Mathias, Stefan; Thumm, Uwe; Mavrikakis, Manos; Aeschlimann, Martin; Oppeneer, Peter M.; Kapteyn, Henry; Murnane, Margaret

    2017-07-01

    Electron-electron interactions are the fastest processes in materials, occurring on femtosecond to attosecond timescales, depending on the electronic band structure of the material and the excitation energy. Such interactions can play a dominant role in light-induced processes such as nano-enhanced plasmonics and catalysis, light harvesting, or phase transitions. However, to date it has not been possible to experimentally distinguish fundamental electron interactions such as scattering and screening. Here, we use sequences of attosecond pulses to directly measure electron-electron interactions in different bands of different materials with both simple and complex Fermi surfaces. By extracting the time delays associated with photoemission we show that the lifetime of photoelectrons from the d band of Cu are longer by ˜100 as compared with those from the same band of Ni. We attribute this to the enhanced electron-electron scattering in the unfilled d band of Ni. Using theoretical modeling, we can extract the contributions of electron-electron scattering and screening in different bands of different materials with both simple and complex Fermi surfaces. Our results also show that screening influences high-energy photoelectrons (≈20 eV) significantly less than low-energy photoelectrons. As a result, high-energy photoelectrons can serve as a direct probe of spin-dependent electron-electron scattering by neglecting screening. This can then be applied to quantifying the contribution of electron interactions and screening to low-energy excitations near the Fermi level. The information derived here provides valuable and unique information for a host of quantum materials.

  6. Technique for the Generation of Attosecond X-Ray Pulses Using an FEL

    CERN Document Server

    Penn, Gregory

    2005-01-01

    We describe a technique for the generation of an isolated burst of X-ray radiation with a duration of ~100 attoseconds in a free electron laser (FEL) employing self-amplified spontaneous emission. Our scheme relies on an initial interaction of the electron beam with an ultra-short laser pulse in a one-period wiggler followed by compression in a dispersive section. The result of this interaction is to create a sub-femtosecond slice of the electron beam with enhanced growth rates for FEL amplification. After many gain lengths through the FEL undulator, the X-ray output from this slice dominates the radiation of the entire bunch. We consider the impact of various effects on the efficiency of this technique. Different configurations are considered in order to realize various timing structures for the resulting radiation.

  7. Attosecond pulse production using resonantly-enhanced high-order harmonics

    CERN Document Server

    Strelkov, V V

    2016-01-01

    We study theoretically the effect of the giant resonance in Xe on the phase difference between the consecutive high order resonantly-enhanced harmonics and calculate the duration of the attosecond pulses produced by these harmonics. For certain conditions resonantly-induced dephasing compensates the phase difference which is intrinsic for the off-resonance harmonics. We find these conditions analytically and compare them with the numerical results. This harmonic synchronization allows attosecond pulse shortening in conjunction with the resonance-induced intensity increase by more than an order of magnitude; the latter enhancement relaxes the requirements for the UV filtering needed for the attosecond pulse production. Using a two-color driving field allows further increase of the intensity. In particular, a caustic-like feature in the harmonic spectrum leads to the generation efficiency growth up to two orders of magnitude, however accompanied by an elongation of the XUV pulse.

  8. Efficient generation of high beam-quality attosecond pulse with polarization-gating Bessel-Gauss beam from highly-ionized media.

    Science.gov (United States)

    Li, Yang; Zhang, Qingbin; Hong, Weiyi; Wang, Shaoyi; Wang, Zhe; Lu, Peixiang

    2012-07-02

    Single attosecond pulse generation with polarization gating Bessel-Gauss beam in relatively strongly-ionized media is investigated. The results show that Bessel-Gauss beam has the ability to suppress the spatial plasma dispersion effects caused by high density of free electrons, thus the laser field can maintain its spatial profile through highly-ionized medium. This indicates the use of Bessel-Gauss beam has advantages over Gaussian beam in high harmonic generation under high ionization conditions. In our scheme, significant improvement of spatiotemporal properties of harmonics is achieved and an isolated attosecond pulse with high beam quality is filtered out using polarization gating.

  9. Generation of bright isolated attosecond soft X-ray pulses driven by multicycle midinfrared lasers.

    Science.gov (United States)

    Chen, Ming-Chang; Mancuso, Christopher; Hernández-García, Carlos; Dollar, Franklin; Galloway, Ben; Popmintchev, Dimitar; Huang, Pei-Chi; Walker, Barry; Plaja, Luis; Jaroń-Becker, Agnieszka A; Becker, Andreas; Murnane, Margaret M; Kapteyn, Henry C; Popmintchev, Tenio

    2014-06-10

    High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest subfemtosecond (attosecond, 10(-18) s) pulses have been produced only in the extreme UV region of the spectrum below 100 eV, which limits the range of materials and molecular systems that can be explored. Here we experimentally demonstrate a remarkable convergence of physics: when midinfrared lasers are used to drive high harmonic generation, the conditions for optimal bright, soft X-ray generation naturally coincide with the generation of isolated attosecond pulses. The temporal window over which phase matching occurs shrinks rapidly with increasing driving laser wavelength, to the extent that bright isolated attosecond pulses are the norm for 2-µm driving lasers. Harnessing this realization, we experimentally demonstrate the generation of isolated soft X-ray attosecond pulses at photon energies up to 180 eV for the first time, to our knowledge, with a transform limit of 35 attoseconds (as), and a predicted linear chirp of 300 as. Most surprisingly, advanced theory shows that in contrast with as pulse generation in the extreme UV, long-duration, 10-cycle, driving laser pulses are required to generate isolated soft X-ray bursts efficiently, to mitigate group velocity walk-off between the laser and the X-ray fields that otherwise limit the conversion efficiency. Our work demonstrates a clear and straightforward approach for robustly generating bright isolated attosecond pulses of electromagnetic radiation throughout the soft X-ray region of the spectrum.

  10. Isolated atto-second pulse generated by spatial shaping of femtosecond laser beam

    Energy Technology Data Exchange (ETDEWEB)

    Strelkov, V.; Mevel, E.; Constant, E. [Univ Bordeaux 1, CELIA, F-33405 Talence (France); Strelkov, V. [Russian Acad Sci, Inst Gen Phys, Moscow 119991 (Russian Federation)

    2009-08-15

    We study numerically the time-dependent HHG phase-matching in the laser beam having a flat-top radial intensity profile. A flat-top profile is the key to produce similar ionization degree at the axis and at the periphery and thus to achieve simultaneous phase-matched generation. Such a profile can be obtained experimentally by using two concentric phase plates that introduce a specific phase shift between the central and the outer part of a focused Gaussian beam. We find realistic laser field parameters and medium density that allow obtaining (after spectral filtering) single atto-second pulse using 10 fs driving laser pulse. Our technique provides isolated atto-second pulse emission almost insensitive on the CEP of the laser pulse. Moreover, the technique is effective both for the mid-plateau and the cut-off spectral range. In particular, the XUV from Ar target in the cut-off spectral range (compatible with the Zr filter) provides isolated atto-second pulse with 185 as duration at a central energy of 92 eV. Using achievable multi mJ 10 fs laser pulses this technique could provide atto-second pulses approaching the {mu}J energy range. (authors)

  11. Attosecond VUV Coherent Control of Molecular Dynamics

    CERN Document Server

    Ranitovic, P; Riviere, P; Palacios, A; Tong, X M; Toshima, N; Gonzalez-Castrillo, A; Martin, L; Martin, F; Murnane, M M; Kapteyn, H C

    2014-01-01

    High harmonic light sources make it possible to access attosecond time-scales, thus opening up the prospect of manipulating electronic wave packets for steering molecular dynamics. However, two decades after the birth of attosecond physics, the concept of attosecond chemistry has not yet been realized. This is because excitation and manipulation of molecular orbitals requires precisely controlled attosecond waveforms in the deep ultraviolet, which have not yet been synthesized. Here, we present a novel approach using attosecond vacuum ultraviolet pulse-trains to coherently excite and control the outcome of a simple chemical reaction in a deuterium molecule in a non-Born Oppenheimer regime. By controlling the interfering pathways of electron wave packets in the excited neutral and singly-ionized molecule, we unambiguously show that we can switch the excited electronic state on attosecond timescales, coherently guide the nuclear wave packets to dictate the way a neutral molecule vibrates, and steer and manipula...

  12. Attosecond light pulses generation along the target surface driven by obliquely-incident lasers

    Science.gov (United States)

    Zhang, Y. X.; Qiao, B.; Xu, X. R.; Chang, H. X.; Zhang, H.; Lu, H. Y.; Yu, M. Y.; Zhou, C. T.; Zhu, S. P.; He, X. T.

    2017-12-01

    A practical approach to achieve strong coherent synchrotron emissions (CSE) in relativistic laser-plasma interaction is proposed, where a plane target with its electron density satisfying the self-similar parameter S ≃ n e 0 / a 0 n c = 1 is obliquely irradiated by a P-polarized laser pulse. In this case, electrons at the target surface are periodically dragged out into the vacuum by the laser field component perpendicular to the target surface, resulting in the formation of a series of dense electron bunches propagating along the target surface. Intense CSE is generated by these electron bunches under acceleration by the laser field component parallel to the target surface. Two-dimensional particle-in-cell simulations show that an intense attosecond light pulse at intensity 9.1 × 1020 W/cm2 (electric field strength ˜41% as that of the drive laser) can be obtained through such CSE. In the high-order harmonics with 15 ω 0 < ω n < 500 ω 0 (ω0 is the laser frequency), the power spectrum of the emission scales as I ( n ) ˜ n - 1.8 and the conversion efficiency from laser to emission reaches ˜10-2.

  13. Attosecond science in atomic, molecular, and condensed matter physics.

    Science.gov (United States)

    Leone, Stephen R; Neumark, Daniel M

    2016-12-16

    Attosecond science represents a new frontier in atomic, molecular, and condensed matter physics, enabling one to probe the exceedingly fast dynamics associated with purely electronic dynamics in a wide range of systems. This paper presents a brief discussion of the technology required to generate attosecond light pulses and gives representative examples of attosecond science carried out in several laboratories. Attosecond transient absorption, a very powerful method in attosecond science, is then reviewed and several examples of gas phase and condensed phase experiments that have been carried out in the Leone/Neumark laboratories are described.

  14. Macroscopic generation of attosecond-pulse trains in strongly ionized media

    Science.gov (United States)

    Tosa, V.; Kim, K. T.; Nam, C. H.

    2009-04-01

    The characteristics of attosecond-pulse trains (APT) obtained from high-order harmonics are investigated by using a nonadiabatic three-dimensional model. A time-dependent phase matching approach is used in order to analyze the macroscopic formation of the APT. Under high ionization conditions, the process of APT formation is found to be the result of an interlace among the driving laser field, single atom response, phase matching effects in the near field and burst interference in the far field.

  15. Fractional high-harmonic combs by attosecond-precision split-spectrum pulse control

    Directory of Open Access Journals (Sweden)

    Laux Martin

    2013-03-01

    Full Text Available Few-cycle laser fields enable pulse-shaping control of high-order harmonic generation by time delaying variable broadband spectral sections. We report the experimental generation of fractional (noninteger high-harmonic combs by the controlled interference of two attosecond pulse trains. Additionally the energy of the high harmonics is strongly tuned with the relative time delay. We quantify the tuning to directly result from the controlled variation of the instantaneous laser frequency at the shaped driver pulse intensity maximum.

  16. Attosecond-controlled photoemission from metal nanowire tips in the few-electron regime

    KAUST Repository

    Ahn, B.

    2017-02-07

    Metal nanotip photoemitters have proven to be versatile in fundamental nanoplasmonics research and applications, including, e.g., the generation of ultrafast electron pulses, the adiabatic focusing of plasmons, and as light-triggered electron sources for microscopy. Here, we report the generation of high energy photoelectrons (up to 160 eV) in photoemission from single-crystalline nanowire tips in few-cycle, 750-nm laser fields at peak intensities of (2-7.3) × 1012 W/cm2. Recording the carrier-envelope phase (CEP)-dependent photoemission from the nanowire tips allows us to identify rescattering contributions and also permits us to determine the high-energy cutoff of the electron spectra as a function of laser intensity. So far these types of experiments from metal nanotips have been limited to an emission regime with less than one electron per pulse. We detect up to 13 e/shot and given the limited detection efficiency, we expect up to a few ten times more electrons being emitted from the nanowire. Within the investigated intensity range, we find linear scaling of cutoff energies. The nonlinear scaling of electron count rates is consistent with tunneling photoemission occurring in the absence of significant charge interaction. The high electron energy gain is attributed to field-induced rescattering in the enhanced nanolocalized fields at the wires apex, where a strong CEP-modulation is indicative of the attosecond control of photoemission.

  17. Attosecond-controlled photoemission from metal nanowire tips in the few-electron regime

    Science.gov (United States)

    Ahn, B.; Schötz, J.; Kang, M.; Okell, W. A.; Mitra, S.; Förg, B.; Zherebtsov, S.; Süßmann, F.; Burger, C.; Kübel, M.; Liu, C.; Wirth, A.; Di Fabrizio, E.; Yanagisawa, H.; Kim, D.; Kim, B.; Kling, M. F.

    2017-03-01

    Metal nanotip photoemitters have proven to be versatile in fundamental nanoplasmonics research and applications, including, e.g., the generation of ultrafast electron pulses, the adiabatic focusing of plasmons, and as light-triggered electron sources for microscopy. Here, we report the generation of high energy photoelectrons (up to 160 eV) in photoemission from single-crystalline nanowire tips in few-cycle, 750-nm laser fields at peak intensities of (2-7.3) × 1012 W/cm2. Recording the carrier-envelope phase (CEP)-dependent photoemission from the nanowire tips allows us to identify rescattering contributions and also permits us to determine the high-energy cutoff of the electron spectra as a function of laser intensity. So far these types of experiments from metal nanotips have been limited to an emission regime with less than one electron per pulse. We detect up to 13 e/shot and given the limited detection efficiency, we expect up to a few ten times more electrons being emitted from the nanowire. Within the investigated intensity range, we find linear scaling of cutoff energies. The nonlinear scaling of electron count rates is consistent with tunneling photoemission occurring in the absence of significant charge interaction. The high electron energy gain is attributed to field-induced rescattering in the enhanced nanolocalized fields at the wires apex, where a strong CEP-modulation is indicative of the attosecond control of photoemission.

  18. Doubly-excited state effects on two-photon double ionization of helium by time-delayed, oppositely circularly-polarized attosecond pulses

    Science.gov (United States)

    Ngoko Djiokap, J. M.; Starace, Anthony F.

    2017-12-01

    We study two-photon double ionization (TPDI) of helium by a pair of time-delayed (non-overlapping), oppositely circularly-polarized attosecond pulses whose carrier frequencies are resonant with 1P o doubly-excited states. All of our TPDI results are obtained by numerical solution of the two-electron time-dependent Schrödinger equation for the six-dimensional case of circularly-polarized attosecond pulses, and they are analyzed using perturbation theory (PT). As compared with the corresponding nonresonant TPDI process, we find that the doubly-excited states change the character of vortex patterns in the two-electron momentum distributions for the case of back-to-back detection of the two ionized electrons in the polarization plane. The doubly-excited states also completely change the structure of fixed-energy, two-electron angular distributions. Moreover, both the fixed-energy and energy-integrated angular distributions, as well as the two-electron energy distributions, exhibit a periodicity with time delay τ between the two attosecond pulses of about 69 as, i.e. the beat period between the (2s2p){}1{{{P}}}o doubly-excited state and the He ground state. Using PT we derive an expression for an angle-integrated energy distribution that is sensitive to the slower beat period ∼1.2 fs between different doubly-excited states as well as to the long timescale ∼17 fs of autoionization lifetimes. However, with our current computer codes we are only able to study numerically the time-dependent phenomena occurring on an attosecond time scale.

  19. Attosecond photoionization dynamics in neon

    DEFF Research Database (Denmark)

    Omiste, Juan J.; Madsen, Lars Bojer

    2018-01-01

    We study the role of electron-electron correlation in the ground-state of Ne, as well as in photoionization dynamics induced by an attosecond XUV pulse. For a selection of central photon energies around 100 eV, we find that while the mean-field time-dependent Hartree-Fock method provides qualitat...

  20. Attosecond streaking of shake-up and Auger electrons in xenon

    Directory of Open Access Journals (Sweden)

    Drescher M.

    2013-03-01

    Full Text Available We present first results of simultaneous attosecond streaking measurements of shake-up electrons and Auger electrons emitted from xenon. We extract relative photo-emission delays for electrons emitted from the 4d, 5s and 5p subshell, as well as for the 5p−25d correlation satellite (shake-up electrons.

  1. Attosecond Electron Correlation Dynamics in Double Ionization of Benzene Probed with Two-Electron Angular Streaking

    Science.gov (United States)

    Winney, Alexander H.; Lee, Suk Kyoung; Lin, Yun Fei; Liao, Qing; Adhikari, Pradip; Basnayake, Gihan; Schlegel, H. Bernhard; Li, Wen

    2017-09-01

    With a novel three-dimensional electron-electron coincidence imaging technique and two-electron angular streaking method, we show that the emission time delay between two electrons can be measured from tens of attoseconds to more than 1 fs. Surprisingly, in benzene, the double ionization rate decays as the time delay between the first and second electron emission increases during the first 500 as. This is further supported by the decay of the Coulomb repulsion in the direction perpendicular to the laser polarization. This result reveals that laser-induced electron correlation plays a major role in strong field double ionization of benzene driven by a nearly circularly polarized field.

  2. Interferometric autocorrelation of an attosecond pulse train in the single-cycle regime.

    Science.gov (United States)

    Nabekawa, Yasuo; Shimizu, Toshihiko; Okino, Tomoya; Furusawa, Kentaro; Hasegawa, Hirokazu; Yamanouchi, Kaoru; Midorikawa, Katsumi

    2006-10-13

    We report on the direct observation of the phase locking of the attosecond pulse train (APT) via interferometric autocorrelation in the extreme ultraviolet region. APT is formed with Fourier synthesis of high-order harmonic fields of a femtosecond laser pulse. Time-of-flight mass spectra of N+, resulting from the Coulomb explosion of N2 absorbing two photons of APT, efficiently yield correlated signals of APT. The measured autocorrelation trace exhibits that the duration of the pulse should be only 1.3 periods of the extreme ultraviolet carrier frequency. A few interference fringes within the short pulse duration clearly show two types of symmetry, which ensure the phase locking between pulses in APT.

  3. Towards optical attosecond pulses: broadband phase coherence between an ultrafast laser and OPO using lock-tozero CEO stabilization

    Directory of Open Access Journals (Sweden)

    Reid D. T.

    2013-03-01

    Full Text Available The carrier-envelope-offset frequencies of the pump, signal, idler and related sum-frequency mixing pulses have been locked to 0 Hz in a 20-fs-Ti:sapphire-pumped optical parametric oscillator, satisfying a critical prerequisite for optical attosecond pulse synthesis.

  4. Attosecond physics at the nanoscale

    CERN Document Server

    Ciappina, M F; Landsman, A S; Okell, W; Zherebtsov, S; Förg, B; Schötz, J; Seiffert, J L; Fennel, T; Shaaran, T; Zimmermann, T; Chacón, A; Guichard, R; Zaïr, A; Tisch, J W G; Marangos, J P; Witting, T; Braun, A; Maier, S A; Roso, L; Krüger, M; Hommelhoff, P; Kling, M F; Krausz, F; Lewenstein, M

    2016-01-01

    Recently two emerging areas of research, attosecond and nanoscale physics, have started to come together. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time scales, interact with atoms, molecules or solids. The laser-induced electron dynamics occurs natively on a timescale down to a few hundred or even tens of attoseconds, which is comparable with the optical field. On the other hand, the second branch involves the manipulation and engineering of mesoscopic systems, such as solids, metals and dielectrics, with nanometric precision. Although nano-engineering is a vast and well-established research field on its own, the merger with intense laser physics is relatively recent. In this article we present a comprehensive experimental and theoretical overview of physics that takes place when short and intense laser pulses interact with nanosystems, such as metallic and dielectric nanostructures. In particular we elucidate how the spati...

  5. Two-photon double ionization of neon using an intense attosecond pulse train

    CERN Document Server

    Manschwetus, B; Campi, F; Maclot, S; Coudert-Alteirac, H; Lahl, J; Wikmark, H; Rudawski, P; Heyl, C M; Farkas, B; Mohamed, T; L'Huillier, A; Johnsson, P

    2016-01-01

    We present the first demonstration of two-photon double ionization of neon using an intense extreme ultraviolet (XUV) attosecond pulse train (APT) in a photon energy regime where both direct and sequential mechanisms are allowed. For an APT generated through high-order harmonic generation (HHG) in argon we achieve a total pulse energy close to 1 $\\mu$J, a central energy of 35 eV and a total bandwidth of $\\sim30$ eV. The APT is focused by broadband optics in a neon gas target to an intensity of $3\\cdot10^{12} $W$\\cdot$cm$^{-2}$. By tuning the photon energy across the threshold for the sequential process the double ionization signal can be turned on and off, indicating that the two-photon double ionization predominantly occurs through a sequential process. The demonstrated performance opens up possibilities for future XUV-XUV pump-probe experiments with attosecond temporal resolution in a photon energy range where it is possible to unravel the dynamics behind direct vs. sequential double ionization and the asso...

  6. Generation of high harmonics and attosecond pulses with ultrashort ...

    Indian Academy of Sciences (India)

    time observation of motion of .... two electron trajectories: a short and a long path, which are the classical counterparts of short and long .... To understand the shearing effect, we analysed the quantum trajectory contributions by means of a ...

  7. Attosecond interferometry with self-amplified spontaneous emission of a free-electron laser

    Science.gov (United States)

    Usenko, Sergey; Przystawik, Andreas; Jakob, Markus Alexander; Lazzarino, Leslie Lamberto; Brenner, Günter; Toleikis, Sven; Haunhorst, Christian; Kip, Detlef; Laarmann, Tim

    2017-05-01

    Light-phase-sensitive techniques, such as coherent multidimensional spectroscopy, are well-established in a broad spectral range, already spanning from radio-frequencies in nuclear magnetic resonance spectroscopy to visible and ultraviolet wavelengths in nonlinear optics with table-top lasers. In these cases, the ability to tailor the phases of electromagnetic waves with high precision is essential. Here we achieve phase control of extreme-ultraviolet pulses from a free-electron laser (FEL) on the attosecond timescale in a Michelson-type all-reflective interferometric autocorrelator. By varying the relative phase of the generated pulse replicas with sub-cycle precision we observe the field interference, that is, the light-wave oscillation with a period of 129 as. The successful transfer of a powerful optical method towards short-wavelength FEL science and technology paves the way towards utilization of advanced nonlinear methodologies even at partially coherent soft X-ray FEL sources that rely on self-amplified spontaneous emission.

  8. EDITORIAL: Focus on Attosecond Physics

    Science.gov (United States)

    Bandrauk, André D.; Krausz, Ferenc; Starace, Anthony F.

    2008-02-01

    Investigations of light-matter interactions and motion in the microcosm have entered a new temporal regime, the regime of attosecond physics. It is a main 'spin-off' of strong field (i.e., intense laser) physics, in which nonperturbative effects are fundamental. Attosecond pulses open up new avenues for time-domain studies of multi-electron dynamics in atoms, molecules, plasmas, and solids on their natural, quantum mechanical time scale and at dimensions shorter than molecular and even atomic scales. These capabilities promise a revolution in our microscopic knowledge and understanding of matter. The recent development of intense, phase-stabilized femtosecond (10-15 s) lasers has allowed unparalleled temporal control of electrons from ionizing atoms, permitting for the first time the generation and measurement of isolated light pulses as well as trains of pulses on the attosecond (1 as = 10-18 s) time scale, the natural time scale of the electron itself (e.g., the orbital period of an electron in the ground state of the H atom is 152 as). This development is facilitating (and even catalyzing) a new class of ultrashort time domain studies in photobiology, photochemistry, and photophysics. These new coherent, sub-fs pulses carried at frequencies in the extreme ultraviolet and soft-x-ray spectral regions, along with their intense, synchronized near-infrared driver waveforms and novel metrology based on sub-fs control of electron-light interactions, are spawning the new science of attosecond physics, whose aims are to monitor, to visualize, and, ultimately, to control electrons on their own time and spatial scales, i.e., the attosecond time scale and the sub-nanometre (Ångstrom) spatial scale typical of atoms and molecules. Additional goals for experiment are to advance the enabling technologies for producing attosecond pulses at higher intensities and shorter durations. According to theoretical predictions, novel methods for intense attosecond pulse generation may in

  9. Relativistic attosecond electron bunch emission from few-cycle laser irradiated nanoscale droplets

    Directory of Open Access Journals (Sweden)

    Laura Di Lucchio

    2015-02-01

    Full Text Available Attosecond electron bunches produced at the surface of nanometer-scale droplets illuminated by a two-cycle laser pulse are investigated for the purpose of determining their optimal emission characteristics. Significant departures from Mie theory are found for electron bunch emission from droplets whose radii satisfy the condition δ_{r}

  10. Attosecond electron-electron collision dynamics of the four-electron escape in Be close to threshold

    CERN Document Server

    Emmanouilidou, A

    2012-01-01

    We explore the escape geometry of four electrons a few eV above threshold following single-photon absorption from the ground state of Be. We find that the four electrons leave the atom on the vertices of a pyramid instead of a previously-predicted tetrahedron. To illustrate the physical mechanisms of quadruple ionization we use a momentum transferring attosecond collision scheme which we show to be in accord with the pyramid break-up pattern.

  11. Connecting Lab-Based Attosecond Science with FEL research

    CERN Multimedia

    CERN. Geneva

    2011-01-01

    In the last few years laboratory-scale femtosecond laser-based research using XUV light has developed dramatically following the successful development of attosecond laser pulses by means of high-harmonic generation. Using attosecond laser pulses, studies of electron dynamics on the natural timescale that electronic processes occur in atoms, molecules and solids can be contemplated, providing unprecedented insight into the fundamental role that electrons play in photo-induced processes. In my talk I will briefly review the present status of the attosecond science research field in terms of present and foreseen capabilities, and discuss a few recent applications, including a first example of the use of attosecond laser pulses in molecular science. In addition, I will discuss very recent results of experiments where photoionization of dynamically aligned molecules is investigated using a high-harmonics XUV source. Photoionization of aligned molecules becomes all the more interesting if the experiment is perfo...

  12. Catching Conical Intersections in the Act; Monitoring Transient Electronic Coherences by Attosecond Stimulated X-Ray Raman Signals

    Science.gov (United States)

    Bennett, Kochise; Kowalewski, Markus; Dorfman, Konstantin; Mukamel, Shaul

    Conical intersections (CIs) dominate the pathways and outcomes of virtually all photochemical molecular processes. Despite extensive experimental and theoretical effort, CIs have not been directly observed yet and the experimental evidence is inferred from fast reaction rates and vibrational signatures. We show that short X-ray pulses can directly detect the passage through a CI with the adequate temporal and spectral sensitivity. The non-adiabatic coupling that exists in the region of a CI redistributes electronic population but also generates electronic coherence. This coherent oscillation can then be detected via a coherent Raman process that employs a composite femtosecond/attosecond X-ray pulse. This technique, dubbed Transient Redistribution of Ultrafast Electronic Coherences (TRUECARS) is reminiscent of Coherent Anti-Stokes Raman Spectroscopy (CARS) in that a coherent oscillation is set in motion and then monitored, but differs in that the dynamics is electronic (CARS generally observes nuclear dynamics) and the coherence is generated internally by passage through a region of non-adiabatic coupling rather than by an externally applied laser. Support provided by U.S. Department of Energy through Award No. DE-FG02-04ER15571, the National Science Foundation (Grant No CHE-1361516), and the Alexander von Humboldt foundation through the Feodor Lynen program.

  13. Attosecond photoionization dynamics in neon

    Science.gov (United States)

    Omiste, Juan J.; Madsen, Lars Bojer

    2018-01-01

    We study the role of electron-electron correlation in the ground state of Ne, as well as in photoionization dynamics induced by an attosecond XUV pulse. For a selection of central photon energies around 100 eV, we find that while the mean-field time-dependent Hartree-Fock method provides qualitatively correct results for the total ionization yield, the photoionization cross section, the photoelectron momentum distribution, as well as for the time delay in photoionization, electron-electron correlation is important for a quantitative description of these quantities.

  14. Attosecond physics at the nanoscale.

    Science.gov (United States)

    Ciappina, M F; Pérez-Hernández, J A; Landsman, A S; Okell, W A; Zherebtsov, S; Förg, B; Schötz, J; Seiffert, L; Fennel, T; Shaaran, T; Zimmermann, T; Chacón, A; Guichard, R; Zaïr, A; Tisch, J W G; Marangos, J P; Witting, T; Braun, A; Maier, S A; Roso, L; Krüger, M; Hommelhoff, P; Kling, M F; Krausz, F; Lewenstein, M

    2017-05-01

    Recently two emerging areas of research, attosecond and nanoscale physics, have started to come together. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time scales, interact with atoms, molecules or solids. The laser-induced electron dynamics occurs natively on a timescale down to a few hundred or even tens of attoseconds (1 attosecond  =  1 as  =  10 -18 s), which is comparable with the optical field. For comparison, the revolution of an electron on a 1s orbital of a hydrogen atom is  ∼152 as. On the other hand, the second branch involves the manipulation and engineering of mesoscopic systems, such as solids, metals and dielectrics, with nanometric precision. Although nano-engineering is a vast and well-established research field on its own, the merger with intense laser physics is relatively recent. In this report on progress we present a comprehensive experimental and theoretical overview of physics that takes place when short and intense laser pulses interact with nanosystems, such as metallic and dielectric nanostructures. In particular we elucidate how the spatially inhomogeneous laser induced fields at a nanometer scale modify the laser-driven electron dynamics. Consequently, this has important impact on pivotal processes such as above-threshold ionization and high-order harmonic generation. The deep understanding of the coupled dynamics between these spatially inhomogeneous fields and matter configures a promising way to new avenues of research and applications. Thanks to the maturity that attosecond physics has reached, together with the tremendous advance in material engineering and manipulation techniques, the age of atto-nanophysics has begun, but it is in the initial stage. We present thus some of the open questions, challenges and prospects for experimental confirmation of theoretical predictions, as well as experiments aimed at characterizing the

  15. Attosecond-correlated dynamics of two electrons in argon

    Indian Academy of Sciences (India)

    2014-01-11

    correlated dynamics of two electrons in argon. V Sharma N Camus B Fischer M Kremer A Rudenko B Bergues M Kuebel N G Johnson M F Kling T Pfeifer J Ullrich R Moshammer. Invited Talks Volume 82 Issue 1 January 2014 ...

  16. Phase distortions of attosecond pulses produced by resonance-enhanced high harmonic generation

    Science.gov (United States)

    Haessler, S.; Strelkov, V.; Elouga Bom, L. B.; Khokhlova, M.; Gobert, O.; Hergott, J.-F.; Lepetit, F.; Perdrix, M.; Ozaki, T.; Salières, P.

    2013-01-01

    Resonant enhancement of high harmonic generation can be obtained in plasmas containing ions with strong radiative transitions resonant with harmonic orders. The mechanism for this enhancement is still debated. We perform the first temporal characterization of the attosecond emission from a tin plasma under near-resonant conditions for two different resonance detunings. We show that the resonance considerably changes the relative phase of neighboring harmonics. For very small detunings, their phase locking may even be lost, evidencing strong phase distortions in the emission process and a modified attosecond structure. These features are well reproduced by our simulations, allowing their interpretation in terms of the phase of the recombination dipole moment.

  17. Theoretical investigation of the isolated attosecond pulse generation by restraining the spatial distribution of high-order harmonic emission

    Science.gov (United States)

    Xia, Chang-Long; Liu, Qi-Ying; Miao, Xiang-Yang

    2018-01-01

    Isolated attosecond pulse (IAP) generation is theoretically investigated by using a few-cycle laser pulse from a two-dimensional model of hydrogen molecular ion. The harmonic spectra from two nuclei of hydrogen molecular ion lead to interference. We investigate the spatial distribution in harmonic generation and propose a scheme to restrain the harmonic generation from the nucleus along the positive-x direction, and thus the interference is weaken in spatial. By using a few-cycle 800 nm chirped laser pulse, the harmonics are mainly generated from the nucleus along negative-x direction in the region of 130th to 230th order. The harmonic spectra are smooth and are mainly contributed by the short quantum path near the cutoff region and IAP with a duration of 97 as is generated. The semiclassical of three-step model is also used to illustrate the physical mechanism.

  18. Attosecond Interference Induced by Coulomb-Field-Driven Transverse Backward-Scattering Electron Wave-Packets

    CERN Document Server

    Song, Xiaohong; Lin, Cheng; Sheng, Zhihao; Yu, Xianhuan; Yang, Weifeng; Hu, Shilin; Chen, Jing; Xu, SongPo; Chen, YongJu; Quan, Wei; Liu, XiaoJun

    2016-01-01

    A novel and universal interference structure is found in the photoelectron momentum distribution of atoms in intense infrared laser field. Theoretical analysis shows that this structure can be attributed to a new form of Coulomb-field-driven backward-scattering of photoelectrons in the direction perpendicular to the laser field, in contrast to the conventional rescattering along the laser polarization direction. This transverse backward-scattering process is closely related to a family of photoelectrons initially ionized within a time interval of less than 200 attosecond around the crest of the laser electric field. Those electrons, acquiring near-zero return energy in the laser field, will be pulled back solely by the ionic Coulomb field and backscattered in the transverse direction. Moreover, this rescattering process mainly occurs at the first or the second return times, giving rise to different phases of the photoelectrons. The interference between these photoelectrons leads to unique curved interference ...

  19. Attosecond Electro-Magnetic Forces Acting on Metal Nanospheres Induced By Relativistic Electrons

    Science.gov (United States)

    Lagos, M. J.; Batson, P. E.; Reyes-Coronado, A.; Echenique, P. M.; Aizpurua, J.

    2014-03-01

    Swift electron scattering near nanoscale materials provides information about light-matter behavior, including induced forces. We calculate time-dependent electromagnetic forces acting on 1-1.5 nm metal nanospheres induced by passing swift electrons, finding both impulse-like and oscillatory response forces. Initially, impulse-like forces are generated by a competition between attractive electric forces and repulsive magnetic forces, lasting a few attoseconds (5-10 as). Oscillatory, plasmonic response forces take place later in time, last a few femtoseconds (1- 5 fs), and apparently rely on photon emission by decay of the electron-induced surface plasmons. A comparison of the strength of these two forces suggests that the impulse-like behavior dominates the process, and can transfer significant linear momentum to the sphere. Our results advance understanding of the physics behind the observation of both attractive and repulsive behavior of gold nano-particles induced by electron beams in aberration-corrected electron microscopy. Work supported under DOE, Award # DE-SC0005132, Basque Gov. project ETORTEK inano, Spanish Ministerio de Ciencia e Innovacion, No. FIS2010-19609-C02-01.

  20. Attosecond lighthouse above 100 eV from high-harmonic generation of mid-infrared pulses

    Science.gov (United States)

    Kovács, K.; Negro, M.; Vozzi, C.; Stagira, S.; Tosa, V.

    2017-10-01

    In this paper, we numerically investigate the possibility to obtain a lighthouse emission for the attosecond pulses produced by high-order harmonics of a strong mid-infrared fundamental pulse without any optical element inserted in the path of the generating beam. The parameters of the driving pulse, focusing geometry, gas medium and detection configuration are currently experimentally feasible. Here, we study in detail the specific propagation conditions of the laser beam, and describe the exact mechanism of the sensitive space-time variation of the medium’s refractive index that lead to the dynamic wavefront rotation. This basic requirement for the lighthouse phenomenon is transmitted to the harmonic bursts, which are emitted with different divergence in successive optical half-cycles, thus can be detected in the far field at increasing distances from the optical axis. In this configuration, spectral filtering of the harmonics is not necessary, therefore the total harmonic pulse power might be used in further pump-probe experiments.

  1. An Attosecond Transient Absorption Spectroscopy Setup with a Water Window Attosecond source

    Science.gov (United States)

    Chew, Andrew; Yin, Yanchun; Li, Jie; Ren, Xiaoming; Wang, Yang; Wu, Yi; Chang, Zenghu

    2017-04-01

    Attosecond transient absorption, or time-resolved pump-probe spectroscopy, are excellent tools that can be used to investigate fast electron dynamics for a given atomic or molecular system. Recent push for high energy long wavelength few cycle laser sources has resulted in the production of x-ray spectra that would allow the probing of electron dynamics at the carbon k-edge in molecules such as CH4 and CO2. The motion of charges can be caused by photo-dissociation and charge migration. We present here the first results from our experimental setup where we produce a broadband attosecond pulse with spectra that stretches into the water window. National Science Foundation (1068604), Army Research Oce (W911NF-14-1-0383), Air Force Oce of Scientic Research (FA9550-15-1-0037, FA9550-16-1-0013) and the DARPA PULSE program by a Grant from AMRDEC (W31P4Q1310017).

  2. Next Generation Driver for Attosecond and Laser-plasma Physics.

    Science.gov (United States)

    Rivas, D E; Borot, A; Cardenas, D E; Marcus, G; Gu, X; Herrmann, D; Xu, J; Tan, J; Kormin, D; Ma, G; Dallari, W; Tsakiris, G D; Földes, I B; Chou, S-W; Weidman, M; Bergues, B; Wittmann, T; Schröder, H; Tzallas, P; Charalambidis, D; Razskazovskaya, O; Pervak, V; Krausz, F; Veisz, L

    2017-07-12

    The observation and manipulation of electron dynamics in matter call for attosecond light pulses, routinely available from high-order harmonic generation driven by few-femtosecond lasers. However, the energy limitation of these lasers supports only weak sources and correspondingly linear attosecond studies. Here we report on an optical parametric synthesizer designed for nonlinear attosecond optics and relativistic laser-plasma physics. This synthesizer uniquely combines ultra-relativistic focused intensities of about 1020 W/cm2 with a pulse duration of sub-two carrier-wave cycles. The coherent combination of two sequentially amplified and complementary spectral ranges yields sub-5-fs pulses with multi-TW peak power. The application of this source allows the generation of a broad spectral continuum at 100-eV photon energy in gases as well as high-order harmonics in relativistic plasmas. Unprecedented spatio-temporal confinement of light now permits the investigation of electric-field-driven electron phenomena in the relativistic regime and ultimately the rise of next-generation intense isolated attosecond sources.

  3. Interaction of relativistic electrons with an intense laser pulse: High-order harmonic generation based on Thomson scattering

    Energy Technology Data Exchange (ETDEWEB)

    Hack, Szabolcs [ELI-ALPS, ELI-HU Non-Profit Ltd., Dugonics tér 13, H-6720 Szeged (Hungary); Department of Theoretical Physics, University of Szeged, Tisza L. krt. 84-86, H-6720 Szeged (Hungary); Varró, Sándor [ELI-ALPS, ELI-HU Non-Profit Ltd., Dugonics tér 13, H-6720 Szeged (Hungary); Wigner Research Center for Physics, SZFI, PO Box 49, H-1525 Budapest (Hungary); Czirják, Attila [ELI-ALPS, ELI-HU Non-Profit Ltd., Dugonics tér 13, H-6720 Szeged (Hungary); Department of Theoretical Physics, University of Szeged, Tisza L. krt. 84-86, H-6720 Szeged (Hungary)

    2016-02-15

    We investigate nonlinear Thomson scattering as a source of high-order harmonic radiation with the potential to enable attosecond light pulse generation. We present a new analytic solution of the electron’s relativistic equations of motion in the case of a short laser pulse with a sine-squared envelope. Based on the single electron emission, we compute and analyze the radiated amplitude and phase spectrum for a realistic electron bunch, with special attention to the correct initial values. These results show that the radiation spectrum of an electron bunch in head-on collision with a sufficiently strong laser pulse of sine-squared envelope has a smooth frequency dependence to allow for the synthesis of attosecond light pulses.

  4. Using the focal phase to control attosecond processes

    Science.gov (United States)

    Hoff, Dominik; Krüger, Michael; Maisenbacher, Lothar; Paulus, Gerhard G.; Hommelhoff, Peter; Sayler, A. M.

    2017-12-01

    The spatial evolution of the electric field of focused broadband light is crucial for many emerging attosecond technologies. Here the effects of the input beam parameters on the evolution of few-cycle laser pulses in the focus are discussed. Specifically, we detail how the frequency-dependent input beam geometry, chirp and chromatic aberration can affect the spatial dependence of the carrier-envelope phase (CEP), central frequency and pulse duration in the focus. These effects are confirmed by a direct, three-dimensional measurement of the CEP-evolution in the focus of a typical few-cycle pulse laser using electron rescattering at metal nanotips in combination with a CEP-metre. Moreover, we demonstrate a simple measurement technique to estimate the focal CEP evolution by input-beam parameters. These parameters can be used in novel ways in order to control attosecond dynamics and tailor highly nonlinear light–matter interactions.

  5. Quantum Chemistry on the time axis: electron correlations and rearrangements on femtosecond and attosecond scales

    CERN Document Server

    Nicolaides, Cleanthes A

    2015-01-01

    Recent developments toward the production and laboratory use of pulses of high intensity, and/or of very high frequency, and/or of ultrashort duration, make possible experiments which can produce time-resolved data on ultrafast transformations involving motions of electrons. The formulation, quantitative understanding and prediction of related new phenomena entail the possibility of computing and applying solutions of the many-electron time-dependent Schroedinger equation, for arbitrary electronic structures, including the dominant effects of Rydberg series, of multiply excited states and of the multi-channel continuous spectrum. To this purpose, we have proposed and applied to many prototypical cases the state-specific expansion approach (SSEA). (Mercouris, Komninos and Nicolaides, Adv. Quantum Chem. 60, 333 (2010)). The paper explains briefly the SSEA, and outlines four of its applications to recently formulated problems concerning time-resolved electronic processes, where electron correlations are crucial....

  6. Attosecond correlation dynamics

    Science.gov (United States)

    Ossiander, M.; Siegrist, F.; Shirvanyan, V.; Pazourek, R.; Sommer, A.; Latka, T.; Guggenmos, A.; Nagele, S.; Feist, J.; Burgdörfer, J.; Kienberger, R.; Schultze, M.

    2017-03-01

    Photoemission of an electron is commonly treated as a one-particle phenomenon. With attosecond streaking spectroscopy we observe the breakdown of this single active-electron approximation by recording up to six attoseconds retardation of the dislodged photoelectron due to electronic correlations. We recorded the photon-energy-dependent emission timing of electrons, released from the helium ground state by an extreme-ultraviolet photon, either leaving the ion in its ground state or exciting it into a shake-up state. We identify an optical field-driven d.c. Stark shift of charge-asymmetric ionic states formed after the entangled photoemission as a key contribution to the observed correlation time shift. These findings enable a complete wavepacket reconstruction and are universal for all polarized initial and final states. Sub-attosecond agreement with quantum mechanical ab initio modelling allows us to determine the absolute zero of time in the photoelectric effect to a precision better than 1/25th of the atomic unit of time.

  7. Probing collective multi-electron effects with few cycle laser pulses

    Science.gov (United States)

    Shiner, Andrew

    High Harmonic Generation (HHG) enables the production of bursts of coherent soft x-rays with attosecond pulse duration. This process arrises from the nonlinear interaction between intense infrared laser pulses and an ionizing gas medium. Soft x-ray photons are used for spectroscopy of inner-shell electron correlation and exchange processes, and the availability of attosecond pulse durations will enable these processes to be resolved on their natural time scales. The maximum or cutoff photon energy in HHG increases with both the intensity as well as the wavelength of the driving laser. It is highly desirable to increase the harmonic cutoff as this will allow for the generation of shorter attosecond pulses, as well as HHG spectroscopy of increasingly energetic electronic transitions. While the harmonic cutoff increases with laser wavelength, there is a corresponding decrease in harmonic yield. The first part of this thesis describes the experimental measurement of the wavelength scaling of HHG efficiency, which we report alambda-6.5+/-1.1 in xenon, and lambda -6.5+/-1.1 in krypton. To increase the HHG cutoff, we have developed a 1.8 microm source, with stable carrier envelope phase and a pulse duration of caries the signature of the electronic structure of the generating medium. In krypton we observed a Cooper minimum at 85 eV, showing that photoionization cross sections can be measured with HHG. Measurements in xenon lead to the first clear observation of electron correlation effects during HHG, which manifest as a broad peak in the HHG spectrum centred at 100 eV. This thesis also describes several improvements to the HHG experiment including the development of an ionization detector for measuring laser intensity, as well as an investigation into the role of laser mode quality on HHG phase matching and efficiency.

  8. Attosecond light sources in the water window

    Science.gov (United States)

    Ren, Xiaoming; Li, Jie; Yin, Yanchun; Zhao, Kun; Chew, Andrew; Wang, Yang; Hu, Shuyuan; Cheng, Yan; Cunningham, Eric; Wu, Yi; Chini, Michael; Chang, Zenghu

    2018-02-01

    As a compact and burgeoning alternative to synchrotron radiation and free-electron lasers, high harmonic generation (HHG) has proven its superiority in static and time-resolved extreme ultraviolet spectroscopy for the past two decades and has recently gained many interests and successes in generating soft x-ray emissions covering the biologically important water window spectral region. Unlike synchrotron and free-electron sources, which suffer from relatively long pulse width or large time jitter, soft x-ray sources from HHG could offer attosecond time resolution and be synchronized with their driving field to investigate time-resolved near edge absorption spectroscopy, which could reveal rich structural and dynamical information of the interrogated samples. In this paper, we review recent progresses on generating and characterizing attosecond light sources in the water window region. We show our development of an energetic, two-cycle, carrier-envelope phase stable laser source at 1.7 μm and our achievement in producing a 53 as soft x-ray pulse covering the carbon K-edge in the water window. Such source paves the ways for the next generation x-ray spectroscopy with unprecedented temporal resolution.

  9. Temporally-coherent terawatt attosecond XFEL synchronized with a few cycle laser.

    Science.gov (United States)

    Kumar, Sandeep; Parc, Yong Woon; Landsman, Alexandra S; Kim, Dong Eon

    2016-11-28

    Attosecond metrology using laser-based high-order harmonics has been significantly advanced and applied to various studies of electron dynamics in atoms, molecules and solids. Laser-based high-order harmonics have a limitation of low power and photon energies. There is, however, a great demand for even higher power and photon energy. Here, we propose a scheme for a terawatt attosecond (TW-as) X-ray pulse in X-ray free-electron laser controlled by a few cycle IR pulse, where one dominant current spike in an electron bunch is used repeatedly to amplify a seeded radiation to a terawatt level. This scheme is relatively simple, compact, straightforward, and also produces a temporally and spectrally clean pulse. The viability of this scheme is demonstrated in simulations using Pohang accelerator laboratory (PAL)-XFEL beam parameters.

  10. Decoherence in attosecond photoionization.

    Science.gov (United States)

    Pabst, Stefan; Greenman, Loren; Ho, Phay J; Mazziotti, David A; Santra, Robin

    2011-02-04

    The creation of superpositions of hole states via single-photon ionization using attosecond extreme-ultraviolet pulses is studied with the time-dependent configuration-interaction singles (TDCIS) method. Specifically, the degree of coherence between hole states in atomic xenon is investigated. We find that interchannel coupling not only affects the hole populations, but it also enhances the entanglement between the photoelectron and the remaining ion, thereby reducing the coherence within the ion. As a consequence, even if the spectral bandwidth of the ionizing pulse exceeds the energy splittings among the hole states involved, perfectly coherent hole wave packets cannot be formed. For sufficiently large spectral bandwidth, the coherence can only be increased by increasing the mean photon energy.

  11. Intensity distributions and isolated attosecond pulse generation from molecular high-order harmonic generation in H2+ driven by nonhomogeneous field

    Science.gov (United States)

    Feng, Liqiang; Chu, Tianshu

    2017-10-01

    Intensity distributions and isolated attosecond pulse generation from the molecular high-order harmonic generation (MHHG) in H2+ and T2+ driven by the nonhomogeneous field have been theoretically investigated. (i) Generally speaking, the intensities of the harmonics driven by the homogeneous field can be enhanced as the initial vibrational state increases and much more intense harmonics can be obtained from the light nuclei. However, with the introduction of the nonhomogeneous effect, the enhanced ratios of the harmonic yields are decreased as the initial vibrational state increases. Moreover, the intensities of the harmonics from H2+ and T2+ are very sensitive to the nonhomogeneous effect of the laser field. (ii) The contributions of the MHHG from the two-H nuclei present the periodic variation as a function of the laser phase for the case of the symmetric nonhomogeneous field. However, for the case of the positive and the negative asymmetric nonhomogeneous fields, the left-H and the right-H play the dominating role in the MHHG, respectively. Moreover, as the angle between the laser polarization direction and the molecular axis increases, the intensity differences of the harmonics from the two-H nuclei are increased. (iii) By properly adding a half-cycle pulse into the positive asymmetric nonhomogeneous field, a supercontinuum with the bandwidth of 279 eV and an isolated 25 as pulse can be obtained.

  12. Compensation of high order harmonic long quantum-path attosecond chirp

    Science.gov (United States)

    Guichard, R.; Caillat, J.; Lévêque, C.; Risoud, F.; Maquet, A.; Taïeb, R.; Zaïr, A.

    2017-12-01

    We propose a method to compensate for the extreme ultra violet (XUV) attosecond chirp associated with the long quantum-path in the high harmonic generation process. Our method employs an isolated attosecond pulse (IAP) issued from the short trajectory contribution in a primary target to assist the infrared driving field to produce high harmonics from the long trajectory in a secondary target. In our simulations based on the resolution of the time-dependent Schrödinger equation, the resulting high harmornics present a clear phase compensation of the long quantum-path contribution, near to Fourier transform limited attosecond XUV pulse. Employing time–frequency analysis of the high harmonic dipole, we found that the compensation is not a simple far-field photonic interference between the IAP and the long-path harmonic emission, but a coherent phase transfer from the weak IAP to the long quantum-path electronic wavepacket. Our approach opens the route to utilizing the long quantum-path for the production and applications of attosecond pulses.

  13. Attosecond Optics and Technology: Progress to Date and Future Prospects [Invited

    Science.gov (United States)

    2016-06-01

    shown to depend on Rabi frequencies with intermediate excited states [116]. Circularly polarized attosecond pulses are theoretically proposed to inves... lattice of 6 pm. The results clearly separate the electronic and nuclear time scales through the experiment. 5. FUTURE PERSPECTIVES The rapid progress in...step-like features in the electronic response, (c) conduction band shift, and (d) slower lattice response. From [119]. Reprinted with permission from

  14. Attosecond dynamics of light-induced resonant hole transfer in high-order-harmonic generation

    Science.gov (United States)

    You, Jhih-An; Dahlström, Jan Marcus; Rohringer, Nina

    2017-02-01

    We present a study of high-order-harmonic generation (HHG) assisted by extreme ultraviolet (XUV) attosecond pulses, which can lead to the excitation of inner-shell electrons and the generation of a second HHG plateau. With the treatment of a one-dimensional model of krypton, based on time-dependent configuration interaction singles (TDCIS) of an effective two-electron system, we show that the XUV-assisted HHG spectrum reveals the duration of the semiclassical electron trajectories. The results are interpreted by the strong-field approximation (SFA) and the importance of the hole transfer during the tunneling process is emphasized. Finally, coherent population transfer between the inner and outer holes with attosecond pulse trains is discussed.

  15. Time-resolved photoemission using attosecond streaking

    Science.gov (United States)

    Nagele, S.; Pazourek, R.; Wais, M.; Wachter, G.; Burgdörfer, J.

    2014-04-01

    We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric efect in the time domain and show that the experimentally accessible time shifts can be decomposed into distinct contributions that stem from the feld-free photoionization process itself and from probe-field induced corrections. We perform accurate quantum-mechanical as well as classical simulations of attosecond streaking for efective one-electron systems and determine all relevant contributions to the time delay with attosecond precision. In particular, we investigate the properties and limitations of attosecond streaking for the transition from short-ranged potentials (photodetachment) to long-ranged Coulomb potentials (photoionization). As an example for a more complex system, we study time-resolved photoionization for endohedral fullerenes A@C60 and discuss how streaking time shifts are modifed due to the interaction of the C60 cage with the probing infrared streaking field.

  16. Probing single-photon ionization on the attosecond time scale

    CERN Document Server

    Klünder, K; Gisselbrecht, M; Fordell, T; Swoboda, M; Guénot, D; Johnsson, P; Caillat, J; Mauritsson, J; Maquet, A; Taïeb, R; L'Huillier, A

    2010-01-01

    We study photoionization of argon atoms excited by attosecond pulses using an interferometric measurement technique. We measure the difference in time delays between electrons emitted from the $3s^2$ and from the $3p^6$ shell, at different excitation energies ranging from 32 to 42 eV. The determination of single photoemission time delays requires to take into account the measurement process, involving the interaction with a probing infrared field. This contribution can be estimated using an universal formula and is found to account for a substantial fraction of the measured delay.

  17. Observation of molecular dipole excitations by attosecond self-streaking

    CERN Document Server

    Wachter, Georg; Sato, Shunsuke A; Pazourek, Renate; Wais, Michael; Lemell, Christoph; Tong, Xiao-Min; Yabana, Kazuhiro; Burgdörfer, Joachim

    2015-01-01

    We propose a protocol to probe the ultrafast evolution and dephasing of coherent electronic excitation in molecules in the time domain by the intrinsic streaking field generated by the molecule itself. Coherent electronic motion in the endohedral fullerene \\Necsixty~is initiated by a moderately intense femtosecond UV-VIS pulse leading to coherent oscillations of the molecular dipole moment that persist after the end of the laser pulse. The resulting time-dependent molecular near-field is probed through the momentum modulation of photoemission from the central neon atom by a time-delayed attosecond XUV pulse. Our ab-initio time-dependent density functional theory and classical trajectory simulations predict that this self-streaking signal accurately traces the molecular dipole oscillations in real time. We discuss the underlying processes and give an analytical model that captures the essence of our ab-initio simulations.

  18. Communication: The electronic structure of matter probed with a single femtosecond hard x-ray pulse

    Directory of Open Access Journals (Sweden)

    J. Szlachetko

    2014-03-01

    Full Text Available Physical, biological, and chemical transformations are initiated by changes in the electronic configuration of the species involved. These electronic changes occur on the timescales of attoseconds (10−18 s to femtoseconds (10−15 s and drive all subsequent electronic reorganization as the system moves to a new equilibrium or quasi-equilibrium state. The ability to detect the dynamics of these electronic changes is crucial for understanding the potential energy surfaces upon which chemical and biological reactions take place. Here, we report on the determination of the electronic structure of matter using a single self-seeded femtosecond x-ray pulse from the Linac Coherent Light Source hard x-ray free electron laser. By measuring the high energy resolution off-resonant spectrum (HEROS, we were able to obtain information about the electronic density of states with a single femtosecond x-ray pulse. We show that the unoccupied electronic states of the scattering atom may be determined on a shot-to-shot basis and that the measured spectral shape is independent of the large intensity fluctuations of the incoming x-ray beam. Moreover, we demonstrate the chemical sensitivity and single-shot capability and limitations of HEROS, which enables the technique to track the electronic structural dynamics in matter on femtosecond time scales, making it an ideal probe technique for time-resolved X-ray experiments.

  19. Attosecond control of optical waveforms

    Energy Technology Data Exchange (ETDEWEB)

    Fuji, Takao [Max-Planck-Institut fuer Quantenoptik, Hans-Kopfermann-Strasse 1, D-85748 Garching (Germany); Rauschenberger, Jens [Max-Planck-Institut fuer Quantenoptik, Hans-Kopfermann-Strasse 1, D-85748 Garching (Germany); Gohle, Christoph [Max-Planck-Institut fuer Quantenoptik, Hans-Kopfermann-Strasse 1, D-85748 Garching (Germany); Apolonski, Alexander [Department fuer Physik, Ludwig-Maximilians-Universitaet Muenchen, Am Coulombwall 1, D-85748 Garching (Germany); Institute of Automation and Electrometry, Russian Academy of Science, 630090 Novosibirsk, Russia (Russian Federation); Udem, Thomas [Max-Planck-Institut fuer Quantenoptik, Hans-Kopfermann-Strasse 1, D-85748 Garching (Germany); Yakovlev, Vladislav S [Department fuer Physik, Ludwig-Maximilians-Universitaet Muenchen, Am Coulombwall 1, D-85748 Garching (Germany); Tempea, Gabriel [Femtolasers Produktions GmbH, Fernkorngasse 10, A-1100 Vienna (Austria); Haensch, Theodor W [Max-Planck-Institut fuer Quantenoptik, Hans-Kopfermann-Strasse 1, D-85748 Garching (Germany); Krausz, Ferenc [Max-Planck-Institut fuer Quantenoptik, Hans-Kopfermann-Strasse 1, D-85748 Garching (Germany); Department fuer Physik, Ludwig-Maximilians-Universitaet Muenchen, Am Coulombwall 1, D-85748 Garching (Germany); Institut fuer Photonik, Technische Universitaet Wien, Gusshausstrasse 27/387, A-1040 Vienna (Austria)

    2005-05-01

    A new, monolithic scheme for stabilizing the phase between the carrier wave and the envelope (CE phase) in a train of few-cycle laser pulses is demonstrated. Self-phase modulation and second-harmonic generation or difference-frequency generation in a single periodically poled lithium niobate crystal, that transmits the main laser beam, allows for the CE-phase locking directly in the usable output. The monolithic scheme obviates the need for splitting off a fraction of the laser output for CE-phase control, coupling into microstructured fibre, as well as separation and recombination of spectral components. As a result, the CE-phase error integrated over the spectral range of 0.2 mHz-35 MHz is as small as 0.016 x 2{pi} rad. This implies that the phase of the field oscillations ({lambda} {approx} 830 nm) with respect to the pulse peak is locked to within 44 attoseconds, resulting in optical waveform control with subhundred attosecond fidelity for the first time.

  20. Photoelectron spectrometer for attosecond spectroscopy of liquids and gases

    Energy Technology Data Exchange (ETDEWEB)

    Jordan, I.; Huppert, M.; Wörner, H. J., E-mail: hwoerner@ethz.ch [Laboratory of Physical Chemistry, ETH Zurich, Vladimir-Prelog-Weg 2, 8093 Zurich (Switzerland); Brown, M. A. [Laboratory for Surface Science and Technology, Department of Materials, ETH Zurich, Vladimir-Prelog-Weg 5, 8093 Zurich (Switzerland); Bokhoven, J. A. van [Institute for Chemical and Bioengineering, ETH Zurich, Vladimir-Prelog-Weg 1, 8093 Zurich (Switzerland); Laboratory for Catalysis and Sustainable Chemistry, Paul Scherrer Institute, 5232 Villigen (Switzerland)

    2015-12-15

    A new apparatus for attosecond time-resolved photoelectron spectroscopy of liquids and gases is described. It combines a liquid microjet source with a magnetic-bottle photoelectron spectrometer and an actively stabilized attosecond beamline. The photoelectron spectrometer permits venting and pumping of the interaction chamber without affecting the low pressure in the flight tube. This pressure separation has been realized through a sliding skimmer plate, which effectively seals the flight tube in its closed position and functions as a differential pumping stage in its open position. A high-harmonic photon spectrometer, attached to the photoelectron spectrometer, exit port is used to acquire photon spectra for calibration purposes. Attosecond pulse trains have been used to record photoelectron spectra of noble gases, water in the gas and liquid states as well as solvated species. RABBIT scans demonstrate the attosecond resolution of this setup.

  1. Progress in sub-femtosecond control of electron localization in ...

    Indian Academy of Sciences (India)

    2014-01-04

    Jan 4, 2014 ... Abstract. Recent advances in controlled generation of intense, ultrashort laser pulses in the ... We discuss the origin of the idea and various ..... generation. 2.3 Electron localization using a combination of many-cycle IR pulse and an attosecond pulse train. Unlike both the above techniques which required ...

  2. Attosecond control of dissociative ionization of O{sub 2} molecules

    Energy Technology Data Exchange (ETDEWEB)

    Siu, W.; Kelkensberg, F.; Gademann, G. [FOM Institute AMOLF, Science Park 104, NL-1098 XG Amsterdam (Netherlands); Rouzee, A.; Vrakking, M. J. J. [FOM Institute AMOLF, Science Park 104, NL-1098 XG Amsterdam (Netherlands); Max-Born-Institut, Max-Born Strasse 2A, D-12489 Berlin (Germany); Johnsson, P. [FOM Institute AMOLF, Science Park 104, NL-1098 XG Amsterdam (Netherlands); Department of Physics, Lund University, Post Office Box 118, SE-221 00 Lund (Sweden); Dowek, D. [Laboratoire des Collisions Atomiques et Moleculaires (UMR Universite Paris-Sud et CNRS, 8625), Batiment 351, Universite Paris-Sud, F-91405 Orsay Cedex (France); Lucchini, M.; Calegari, F. [Department of Physics, Politecnico di Milano, Istituto di Fotonica e Nanotecnologie CNR-IFN, Piazza Leonardo da Vinci 32, 20133 Milano (Italy); De Giovannini, U.; Rubio, A. [Nano-bio Spectroscopy Group, ETSF Scientific Development Centre, Universidad del Pais Vasco, Avenida Tolosa 72, E-20018 San Sebastian (Spain); Lucchese, R. R. [Department of Chemistry, Texas A and M University, Post Office Box 30012, College Station, Texas 77842-3012 (United States); Kono, H. [Department of Chemistry, Graduate School of Science, Tohoku University, Sendai 980-8578 (Japan); Lepine, F. [Universite Lyon 1/CNRS/LASIM, UMR 5579, 43 Boulevard Du 11 Novembre 1918, F-69622 Villeurbane (France)

    2011-12-15

    We demonstrate that dissociative ionization of O{sub 2} can be controlled by the relative delay between an attosecond pulse train (APT) and a copropagating infrared (IR) field. Our experiments reveal a dependence of both the branching ratios between a range of electronic states and the fragment angular distributions on the extreme ultraviolet (XUV) to IR time delay. The observations go beyond adiabatic propagation of dissociative wave packets on IR-induced quasistatic potential energy curves and are understood in terms of an IR-induced coupling between electronic states in the molecular ion.

  3. Light field driven streak-camera for single-shot measurements of the temporal profile of XUV-pulses from a free-electron laser; Lichtfeld getriebene Streak-Kamera zur Einzelschuss Zeitstrukturmessung der XUV-Pulse eines Freie-Elektronen Lasers

    Energy Technology Data Exchange (ETDEWEB)

    Fruehling, Ulrike

    2009-10-15

    The Free Electron Laser in Hamburg (FLASH) is a source for highly intense ultra short extreme ultraviolet (XUV) light pulses with pulse durations of a few femtoseconds. Due to the stochastic nature of the light generation scheme based on self amplified spontaneous emission (SASE), the duration and temporal profile of the XUV pulses fluctuate from shot to shot. In this thesis, a THz-field driven streak-camera capable of single pulse measurements of the XUV pulse-profile has been realized. In a first XUV-THz pump-probe experiment at FLASH, the XUV-pulses are overlapped in a gas target with synchronized THz-pulses generated by a new THz-undulator. The electromagnetic field of the THz light accelerates photoelectrons produced by the XUV-pulses with the resulting change of the photoelectron momenta depending on the phase of the THz field at the time of ionisation. This technique is intensively used in attosecond metrology where near infrared streaking fields are employed for the temporal characterisation of attosecond XUV-Pulses. Here, it is adapted for the analysis of pulse durations in the few femtosecond range by choosing a hundred times longer far infrared streaking wavelengths. Thus, the gap between conventional streak cameras with typical resolutions of hundreds of femtoseconds and techniques with attosecond resolution is filled. Using the THz-streak camera, the time dependent electric field of the THz-pulses was sampled in great detail while on the other hand the duration and even details of the time structure of the XUV-pulses were characterized. (orig.)

  4. Transient Impulsive Giant Electronic Raman Redistribution

    CERN Document Server

    Miyabe, S

    2014-01-01

    Resonant Raman excitation by ultrafast vacuum ultraviolet laser pulses is a powerful means to study electron dynamics in molecules, but experiments must contend with linear background ionization: frequencies high enough to reach resonant core-valence transitions will usually ionize all occupied orbitals as well, and the ionization cross sections are usually dominant. Here we show that attosecond pulses can induce a new process, transient impulsive stimulated Raman scattering, which can overwhelm valence ionization. Calculations are performed for atomic sodium, but the principal is valid for many molecular systems. This approach opens the path for high fidelity multidimensional spectroscopy with attosecond pulses.

  5. Coherent pump pulses in Double Electron Electron Resonance Spectroscopy

    Science.gov (United States)

    Tait, Claudia E.; Stoll, Stefan

    2016-01-01

    The recent introduction of shaped pulses to Double Electron Electron Resonance (DEER) spectroscopy has led to significant enhancements in sensitivity through increased excitation bandwidths and improved control over spin dynamics. The application of DEER has so far relied on the presence of an incoherent pump channel to average out most undesired coherent effects of the pump pulse(s) on the observer spins. However, in fully coherent EPR spectrometers that are increasingly used to generate shaped pulses, the presence of coherent pump pulses means that these effects need to be explicitly considered. In this paper, we examine the effects of coherent rectangular and sech/tanh pump pulses in DEER experiments with up to three pump pulses. We show that, even in the absence of significant overlap of the observer and pump pulse excitation bandwidths, coherence transfer pathways involving both types of pulses generate spin echoes of considerable intensity. These echoes introduce artefacts, which, if not identified and removed, can easily lead to misinterpretation. We demonstrate that the observed echoes can be quantitatively modelled using a simple spin quantum dynamics approach that includes instrumental transfer functions. Based on an analysis of the echo crossing artefacts, we propose efficient phase cycling schemes for their suppression. This enables the use of advanced DEER experiments, characterized by high sensitivity and increased accuracy for long-distance measurements, on novel fully coherent EPR spectrometers. PMID:27339858

  6. Attosecond experiments on plasmonic nanostructures principles and experiments

    CERN Document Server

    Schötz, Johannes

    2016-01-01

    Johannes Schötz presents the first measurements of optical electro-magnetic near-fields around nanostructures with subcycle-resolution. The ability to measure and understand light-matter interactions on the nanoscale is an important component for the development of light-wave-electronics, the control and steering of electron dynamics with the frequency of light, which promises a speed-up by several orders of magnitude compared to conventional electronics. The experiments presented here on metallic nanotips, widely used in experiments and applications, do not only demonstrate the feasibility of attosecond streaking as a unique tool for fundamental studies of ultrafast nanophotonics but also represent a first important step towards this goal. Contents Electron Scattering in Solids Attosecond Streaking from Metal Nanotips Target Groups Lecturers and students of physics, especially in the area of nanophotonics and attosecond physics About the Author Johannes Schötz received his Master's degree in physics and cu...

  7. Controlling electronic couplings with tunable long wavelength pulses: Study of Autler-Townes splitting and XUV emission spectra

    Science.gov (United States)

    Harkema, Nathan; Liao, Chen-Ting; Sandhu, Arvinder

    2017-04-01

    Attosecond transient absorption spectroscopy (ATAS) enables the study of excited electron dynamics with unprecedented temporal and energy resolution. Many ATAS experiments use an extreme ultraviolet (XUV) pump pulse and a near-infrared (NIR) probe fixed at the fundamental laser frequency ( 800 nm) to study the light induced effects on electronic structure of atoms and molecules. We extend the technique by using an optical parametric amplifier in one arm of our setup, which allows us to independently tune the frequency of the probe pulse from 1200 to 1800 nm. These long-wavelength pulses allow us to explore a new regime, where we can control the couplings between nearby electronic states to alter the transient absorption lineshapes in atoms. We use this technique to investigate the 4p-3s detuning dependent Autler-Townes splitting of the 4p state in Helium. Light induced Floquet structures extending into the continuum are observed in our study. We demonstrate new tunable XUV emission channels from four-wave mixing processes, and the efficiency of these emissions can be strongly enhanced through resonant couplings. The tunable IR induced electronic couplings are also used to influence the autoionization dynamics in Argon. This work is supported by NSF Grant No. PHY-1505556 and ARO Grant No. W911NF-14-1-0383.

  8. Zeptosecond precision pulse shaping.

    Science.gov (United States)

    Köhler, Jens; Wollenhaupt, Matthias; Bayer, Tim; Sarpe, Cristian; Baumert, Thomas

    2011-06-06

    We investigate the temporal precision in the generation of ultrashort laser pulse pairs by pulse shaping techniques. To this end, we combine a femtosecond polarization pulse shaper with a polarizer and employ two linear spectral phase masks to mimic an ultrastable common-path interferometer. In an all-optical experiment we study the interference signal resulting from two temporally delayed pulses. Our results show a 2σ-precision of 300 zs = 300 × 10(-21) s in pulse-to-pulse delay. The standard deviation of the mean is 11 zs. The obtained precision corresponds to a variation of the arm's length in conventional delay stage based interferometers of 0.45 Å. We apply these precisely generated pulse pairs to a strong-field quantum control experiment. Coherent control of ultrafast electron dynamics via photon locking by temporal phase discontinuities on a few attosecond timescale is demonstrated.

  9. Attosecond pre-determination of reaction dynamics in polyatomic molecules

    Science.gov (United States)

    Kitzler, Markus

    2014-05-01

    An important aim of Ultrafast Laser Science and Attosecond Physics is the measurement of valence electron dynamics in molecules during complex restructuring and fragmentation reactions. Such reactions may be triggered by the removal of electrons, e.g., by ionization with intense, ultrashort laser pulses. Depending on the valence-shell from which the electrons are removed, the molecular ion might be put into a binding state or a certain dissociative state. With control over the ionization process it might thus be possible to gain control over the subsequent restructuring and fragmentation processes on a purely electronic level. Detailed insight into the process of electron removal can be obtained from interferometric measurements using two bound state wavepackets released at different times within a sub-cycle of a laser field. I will present results of experiments that exploit this kind of electron wavepacket interferometry with sub-10 attosecond resolution for tracing the evolution of the phase of the bound state of an atom or molecule during the removal of an electron. I will furthermore present two conceptually similar schemes that allow pre-determining the outcome of molecular restructuring and fragmentation processes in polyatomic molecules on sub-femtosecond time-scales by gaining control over the process of electron removal. The first method involves recollision double ionization in intense few-cycle laser fields with a known carrier-envelope phase (CEP). Tuning of the CEP allows controlling the removal of inner-valence electrons and the controlled population of dissociative excited states. Using this method I will show experimental CEP-control over various fragmentation reactions of a series of polyatomic molecules. The second control scheme uses the strong preponderance of ionization from specific molecular orbitals to the alignment of the molecular axis with respect to the laser polarization direction for determining which valence level the electrons are

  10. Development of extreme ultraviolet and soft x-ray multilayer optics for scientific studies with femtosecond/attosecond sources

    Energy Technology Data Exchange (ETDEWEB)

    Aquila, Andrew Lee [Univ. of California, Berkeley, CA (United States)

    2009-05-21

    The development of multilayer optics for extreme ultraviolet (EUV) radiation has led to advancements in many areas of science and technology, including materials studies, EUV lithography, water window microscopy, plasma imaging, and orbiting solar physics imaging. Recent developments in femtosecond and attosecond EUV pulse generation from sources such as high harmonic generation lasers, combined with the elemental and chemical specificity provided by EUV radiation, are opening new opportunities to study fundamental dynamic processes in materials. Critical to these efforts is the design and fabrication of multilayer optics to transport, focus, shape and image these ultra-fast pulses This thesis describes the design, fabrication, characterization, and application of multilayer optics for EUV femtosecond and attosecond scientific studies. Multilayer mirrors for bandwidth control, pulse shaping and compression, tri-material multilayers, and multilayers for polarization control are described. Characterization of multilayer optics, including measurement of material optical constants, reflectivity of multilayer mirrors, and metrology of reflected phases of the multilayer, which is critical to maintaining pulse size and shape, were performed. Two applications of these multilayer mirrors are detailed in the thesis. In the first application, broad bandwidth multilayers were used to characterize and measure sub-100 attosecond pulses from a high harmonic generation source and was performed in collaboration with the Max-Planck institute for Quantum Optics and Ludwig- Maximilians University in Garching, Germany, with Professors Krausz and Kleineberg. In the second application, multilayer mirrors with polarization control are useful to study femtosecond spin dynamics in an ongoing collaboration with the T-REX group of Professor Parmigiani at Elettra in Trieste, Italy. As new ultrafast x-ray sources become available, for example free electron lasers, the multilayer designs

  11. Attosecond delays in laser-assisted photodetachment from closed-shell negative ions

    Science.gov (United States)

    Lindroth, Eva; Dahlström, Jan Marcus

    2017-07-01

    We study laser-assisted photodetachment time delays by attosecond pulse trains from the closed-shell negative ions F- and Cl-. We investigate the separability of the delay into two contributions: (i) the Wigner-like delay associated with one-photon ionization by the attosecond pulse train and (ii) the delay associated with the exchange of an additional laser photon in the presence of the potential of the remaining target. Based on the asymptotic form of the wave packet, the latter term is expected to be negligible because the ion is neutralized, leading to a vanishing laser-ion interaction with increasing electron-atom separation. While this asymptotic behavior is verified at high photoelectron energies, we also quantify sharp deviations at low photoelectron energies. Further, these low-energy delays are clearly different for the two studied anions, indicating a breakdown of the universality of laser-ion-induced delays. The fact that the short-range potential can induce a delay of as much as 50 as can have implications for the interpretation of delay measurements also in other systems that lack long-range potential.

  12. Can strong-field ionization prepare attosecond dynamics?

    CERN Document Server

    Pabst, Stefan

    2015-01-01

    Strong-field ionization (SFI) has been shown to prepare wave packets with few-femtosecond periods. Here, we explore whether this technique can be extended to the attosecond time scale. We introduce an intuitive model for predicting the bandwidth of ionic states that can be coherently prepared by SFI. This bandwidth is given by the Fourier-transformed sub-cycle SFI rate and decreases considerably with increasing central wavelength of the ionizing pulse. Many-body calculations based on time-dependent configuration-interaction singles (TDCIS) quantitatively support this result and reveal an additional decrease of the bandwidth as a consequence of channel interactions and non-adiabatic dynamics. Our results further predict that multi-cycle femtosecond pulses can coherently prepare attosecond wave packets with higher selectivity and versatility compared to single-cycle pulses.

  13. Theory of attosecond absorption spectroscopy in krypton

    DEFF Research Database (Denmark)

    Baggesen, Jan Conrad; Lindroth, Eva; Madsen, Lars Bojer

    2012-01-01

    A theory for time-domain attosecond pump–attosecond probe photoabsorption spectroscopy is formulated and related to the atomic response. The theory is illustrated through a study of attosecond absorption spectroscopy in krypton. The atomic parameters entering the formulation such as energies...

  14. Modulation of attosecond beating in resonant two-photon ionization

    CERN Document Server

    Galán, Álvaro J; Martín, Fernando

    2014-01-01

    We present a theoretical study of the photoelectron attosecond beating at the basis of RABBIT (Reconstruction of Attosecond Beating By Interference of Two-photon transitions) in the presence of autoionizing states. We show that, as a harmonic traverses a resonance, its sidebands exhibit a peaked phase shift as well as a modulation of the beating frequency itself. Furthermore, the beating between two resonant paths persists even when the pump and the probe pulses do not overlap, thus providing a sensitive non-holographic interferometric means to reconstruct coherent metastable wave packets. We characterize these phenomena quantitatively with a general finite-pulse analytical model that accounts for the effect of both intermediate and final resonances on two-photon processes, at a negligible computational cost. The model predictions are in excellent agreement with those of accurate ab initio calculations for the helium atom in the region of the N=2 doubly excited states.

  15. Accuracy of laser measurements improved by pulse autocorrelator electronic system

    Science.gov (United States)

    Campanella, S. J.

    1967-01-01

    Pulse autocorrelator electronic system discriminates between the dispersion effect of a disturbed laser signal and background noise by detecting multipath arrivals of Gaussian-shaped signal pulses. The autocorrelation function is time-dependent and can be determined by integrating the product of a received pulse and its delayed replicas.

  16. Progress in sub-femtosecond control of electron localization in ...

    Indian Academy of Sciences (India)

    2014-01-04

    Jan 4, 2014 ... Recent advances in controlled generation of intense, ultrashort laser pulses in the femtosecond and attosecond time-scales have pushed new avenues of research in the coherent control of ... We discuss the origin of the idea and various mechanisms to achieve electron localization in small molecules.

  17. CTS and CZTS for solar cells made by pulsed laser deposition and pulsed electron deposition

    DEFF Research Database (Denmark)

    Ettlinger, Rebecca Bolt

    This thesis concerns the deposition of thin films for solar cells using pulsed laser deposition (PLD) and pulsed electron deposition (PED). The aim was to deposit copper tin sulfide (CTS) and zinc sulfide (ZnS) by pulsed laser deposition to learn about these materials in relation to copper zinc tin......, which make them promising alternatives to the commercially successful solar cell material copper indium gallium diselenide (CIGS). Complementing our group's work on pulsed laser deposition of CZTS, we collaborated with IMEM-CNR in Parma, Italy, to deposit CZTS by pulsed electron deposition for the first...... of using pulsed electron deposition was to make CZTS at a low processing temperature, avoiding the 570 °C annealing step used for our pulsed laser deposited solar cells. Preliminary solar cells had an efficiency of 0.2 % with a 300 °C deposition step without annealing. Further process control is needed...

  18. Attosecond beamline with actively stabilized and spatially separated beam paths.

    Science.gov (United States)

    Huppert, M; Jordan, I; Wörner, H J

    2015-12-01

    We describe a versatile and compact beamline for attosecond spectroscopy. The setup consists of a high-order harmonic source followed by a delay line that spatially separates and then recombines the extreme-ultraviolet (XUV) and residual infrared (IR) pulses. The beamline introduces a controlled and actively stabilized delay between the XUV and IR pulses on the attosecond time scale. A new active-stabilization scheme combining a helium-neon-laser and a white-light interferometer minimizes fluctuations and allows to control delays accurately (26 as rms during 1.5 h) over long time scales. The high-order-harmonic-generation region is imaged via optical systems, independently for XUV and IR, into an interaction volume to perform pump-probe experiments. As a consequence of the spatial separation, the pulses can be independently manipulated in intensity, polarization, and frequency content. The beamline can be combined with a variety of detectors for measuring attosecond dynamics in gases, liquids, and solids.

  19. Optimizing chirped laser pulse parameters for electron acceleration in vacuum

    Energy Technology Data Exchange (ETDEWEB)

    Akhyani, Mina; Jahangiri, Fazel; Niknam, Ali Reza; Massudi, Reza, E-mail: r-massudi@sbu.ac.ir [Laser and Plasma Research Institute, Shahid Beheshti University, Tehran 1983969411 (Iran, Islamic Republic of)

    2015-11-14

    Electron dynamics in the field of a chirped linearly polarized laser pulse is investigated. Variations of electron energy gain versus chirp parameter, time duration, and initial phase of laser pulse are studied. Based on maximizing laser pulse asymmetry, a numerical optimization procedure is presented, which leads to the elimination of rapid fluctuations of gain versus the chirp parameter. Instead, a smooth variation is observed that considerably reduces the accuracy required for experimentally adjusting the chirp parameter.

  20. Attosecond Timing in Optical-to-Electrical Conversion

    CERN Document Server

    Baynes, Fred N; Fortier, Tara; Zhou, Qiugui; Beling, Andreas; Campbell, Joe C; Diddames, Scott A

    2014-01-01

    The most frequency-stable sources of electromagnetic radiation are produced optically, and optical frequency combs provide the means for high fidelity frequency transfer across hundreds of terahertz and into the microwave domain. A critical step in this photonic-based synthesis of microwave signals is the optical-to-electrical conversion process. Here we show that attosecond (as) timing stability can be preserved across the opto-electronic interface of a photodiode, despite an intrinsic temporal response that is more than six orders of magnitude slower. The excess timing noise in the photodetection of a periodic train of ultrashort optical pulses behaves as flicker noise (1/f) with amplitude of 4 as/Sqrt(Hz) at 1 Hz offset. The corresponding fractional frequency fluctuations are 1.4x10-17 at 1 second and 5.5x10-20 at 1000 seconds. These results demonstrate that direct photodetection, as part of frequency-comb-based microwave synthesis, can support the timing performance of the best optical frequency standards...

  1. Two-pulse laser control of nuclear and electronic motion

    DEFF Research Database (Denmark)

    Grønager, Michael; Henriksen, Niels Engholm

    1997-01-01

    We discuss an explicitly time-dependent two-pulse laser scheme for controlling where nuclei and electrons are going in unimolecular reactions. We focus on electronic motion and show, with HD+ as an example, that one can find non-stationary states where the electron (with some probability) oscilla......We discuss an explicitly time-dependent two-pulse laser scheme for controlling where nuclei and electrons are going in unimolecular reactions. We focus on electronic motion and show, with HD+ as an example, that one can find non-stationary states where the electron (with some probability...

  2. A novel programmable pulse generator with nanosecond resolution for pulsed electron paramagnetic resonance applications.

    Science.gov (United States)

    Devasahayam, N; Subramanian, S; Krishna, M C

    2008-02-01

    A pulse programmer with nanosecond time resolution needed for time-domain electron paramagnetic resonance (EPR) spectroscopic applications is described. This unit uses commercially available timing and input-output port modules and control software developed in our laboratory. The pulse programmer is operated through a personal computer front panel graphic user interface (GUI) inputs to control pulse widths, delays, and the associated acquisition trigger timings. Based on these parameters, all other associated gate and trigger timings are internally generated automatically without the need to enter them explicitly. The excitation pulse widths were of nanosecond resolution while all other gate pulses can be incremented in steps of 20 ns without compromising spectrometer performance. In the current configuration, the pulse programmer permits generation of a single pulse or multiple pulse sequences for EPR imaging with minimal data entry via the front panel GUI.

  3. Helicity-Selective Phase-Matching and Quasi-Phase matching of Circularly Polarized High-Order Harmonics: Towards Chiral Attosecond Pulses

    Science.gov (United States)

    2016-05-23

    linearly polarized, the recollision (and recombination) probability is high since the trajectory of the electron is linear. This ‘head on’ recollision...yields linearly polarized HHG bursts. Introducing ellipticity into the driving laser field results in the generation of elliptically polarized harmonics...23–25]. However, in this case the HHG efficiency drops drastically since the electron trajectory misses the parent ion [26]. Although many theoretical

  4. Electron pulse shaping in the FELIX RF accelerator

    NARCIS (Netherlands)

    Weits, H. H.; van der Geer, C. A. J.; Oepts, D.; van der Meer, A. F. G.

    1999-01-01

    The FELIX free-electron laser uses short pulses of relativistic electrons produced by an RF accelerator. The design target for the duration of these electron bunches was around 3 ps. In experiments we observed that the bunches emit coherently enhanced spontaneous emission (CSE) when they travel

  5. Compact pulsed electron beam system for microwave generation

    Science.gov (United States)

    Sharma, S. K.; Deb, P.; Shukla, R.; Banerjee, P.; Prabaharan, T.; Adhikary, B.; Verma, R.; Sharma, A.; Shyam, A.

    2012-11-01

    A compact 180 kV electron beam system is designed for high power microwave generation. The electron beam system is consists of a secondary energy storage device, which can deliver energy to the load at faster rate than usual primary energy storage system such as tesla transformers or marx generator. The short duration, high voltage pulse with fast rise time and good flattop is applied to vacuum diode for high power microwave generation. The compact electron beam system is made up of single turn primary tesla transformer which charges a helical pulse forming line and transfers its energy to vacuum diode through a high voltage pressurized spark gap switch. We have used helical pulse forming line which has higher inductance as compared to coaxial pulse forming line, which in turns increases, the pulse width and reduce the length of the pulse forming line. Water dielectric medium is used because of its high dielectric constant, high dielectric strength and efficient energy storage capability. The time dependent breakdown property and high relative permittivity of water makes it an ideal choice for this system. The high voltage flat-top pulse of 90 kV, 260 ns is measured across the matched load. In this article we have reported the design details, simulation and initial experimental results of 180 kV pulsed electron beam system for high power microwave generation.

  6. Electromagnetic solitary pulses in a magnetized electron-positron plasma.

    Science.gov (United States)

    Shukla, P K; Eliasson, B; Stenflo, L

    2011-09-01

    A theory for large amplitude compressional electromagnetic solitary pulses in a magnetized electron-positron (e-p) plasma is presented. The pulses, which propagate perpendicular to the external magnetic field, are associated with the compression of the plasma density and the wave magnetic field. Here the solitary wave magnetic field pressure provides the restoring force, while the inertia comes from the equal mass electrons and positrons. The solitary pulses are formed due to a balance between the compressional wave dispersion arising from the curl of the inertial forces in Faraday's law and the nonlinearities associated with the divergence of the electron and positron fluxes, the nonlinear Lorentz forces, the advection of the e-p fluids, and the nonlinear plasma current densities. The compressional solitary pulses can exist in a well-defined speed range above the Alfvén speed. They can be associated with localized electromagnetic field excitations in magnetized laboratory and space plasmas composed of electrons and positrons.

  7. AXSIS: Exploring the frontiers in attosecond X-ray science, imaging and spectroscopy

    Science.gov (United States)

    Kärtner, F. X.; Ahr, F.; Calendron, A.-L.; Çankaya, H.; Carbajo, S.; Chang, G.; Cirmi, G.; Dörner, K.; Dorda, U.; Fallahi, A.; Hartin, A.; Hemmer, M.; Hobbs, R.; Hua, Y.; Huang, W. R.; Letrun, R.; Matlis, N.; Mazalova, V.; Mücke, O. D.; Nanni, E.; Putnam, W.; Ravi, K.; Reichert, F.; Sarrou, I.; Wu, X.; Yahaghi, A.; Ye, H.; Zapata, L.; Zhang, D.; Zhou, C.; Miller, R. J. D.; Berggren, K. K.; Graafsma, H.; Meents, A.; Assmann, R. W.; Chapman, H. N.; Fromme, P.

    2016-09-01

    -, accelerator,- X-ray scientists as well as spectroscopists and biochemists optimizes X-ray pulse parameters, in tandem with sample delivery, crystal size, and advanced X-ray detectors. Ultimately, the new capability, attosecond serial X-ray crystallography and spectroscopy, will be applied to one of the most important problems in structural biology, which is to elucidate the dynamics of light reactions, electron transfer and protein structure in photosynthesis.

  8. Pulse Duration of Seeded Free-Electron Lasers

    Science.gov (United States)

    Finetti, Paola; Höppner, Hauke; Allaria, Enrico; Callegari, Carlo; Capotondi, Flavio; Cinquegrana, Paolo; Coreno, Marcello; Cucini, Riccardo; Danailov, Miltcho B.; Demidovich, Alexander; De Ninno, Giovanni; Di Fraia, Michele; Feifel, Raimund; Ferrari, Eugenio; Fröhlich, Lars; Gauthier, David; Golz, Torsten; Grazioli, Cesare; Kai, Yun; Kurdi, Gabor; Mahne, Nicola; Manfredda, Michele; Medvedev, Nikita; Nikolov, Ivaylo P.; Pedersoli, Emanuele; Penco, Giuseppe; Plekan, Oksana; Prandolini, Mark J.; Prince, Kevin C.; Raimondi, Lorenzo; Rebernik, Primoz; Riedel, Robert; Roussel, Eleonore; Sigalotti, Paolo; Squibb, Richard; Stojanovic, Nikola; Stranges, Stefano; Svetina, Cristian; Tanikawa, Takanori; Teubner, Ulrich; Tkachenko, Victor; Toleikis, Sven; Zangrando, Marco; Ziaja, Beata; Tavella, Franz; Giannessi, Luca

    2017-04-01

    The pulse duration, and, more generally, the temporal intensity profile of free-electron laser (FEL) pulses, is of utmost importance for exploring the new perspectives offered by FELs; it is a nontrivial experimental parameter that needs to be characterized. We measured the pulse shape of an extreme ultraviolet externally seeded FEL operating in high-gain harmonic generation mode. Two different methods based on the cross-correlation of the FEL pulses with an external optical laser were used. The two methods, one capable of single-shot performance, may both be implemented as online diagnostics in FEL facilities. The measurements were carried out at the seeded FEL facility FERMI. The FEL temporal pulse characteristics were measured and studied in a range of FEL wavelengths and machine settings, and they were compared to the predictions of a theoretical model. The measurements allowed a direct observation of the pulse lengthening and splitting at saturation, in agreement with the proposed theory.

  9. Quantum coherent optical phase modulation in an ultrafast transmission electron microscope.

    Science.gov (United States)

    Feist, Armin; Echternkamp, Katharina E; Schauss, Jakob; Yalunin, Sergey V; Schäfer, Sascha; Ropers, Claus

    2015-05-14

    Coherent manipulation of quantum systems with light is expected to be a cornerstone of future information and communication technology, including quantum computation and cryptography. The transfer of an optical phase onto a quantum wavefunction is a defining aspect of coherent interactions and forms the basis of quantum state preparation, synchronization and metrology. Light-phase-modulated electron states near atoms and molecules are essential for the techniques of attosecond science, including the generation of extreme-ultraviolet pulses and orbital tomography. In contrast, the quantum-coherent phase-modulation of energetic free-electron beams has not been demonstrated, although it promises direct access to ultrafast imaging and spectroscopy with tailored electron pulses on the attosecond scale. Here we demonstrate the coherent quantum state manipulation of free-electron populations in an electron microscope beam. We employ the interaction of ultrashort electron pulses with optical near-fields to induce Rabi oscillations in the populations of electron momentum states, observed as a function of the optical driving field. Excellent agreement with the scaling of an equal-Rabi multilevel quantum ladder is obtained, representing the observation of a light-driven 'quantum walk' coherently reshaping electron density in momentum space. We note that, after the interaction, the optically generated superposition of momentum states evolves into a train of attosecond electron pulses. Our results reveal the potential of quantum control for the precision structuring of electron densities, with possible applications ranging from ultrafast electron spectroscopy and microscopy to accelerator science and free-electron lasers.

  10. Multiple pulse electron beam converter design for high power radiography

    Science.gov (United States)

    Pincosy, P. A.; Back, N.; Bergstrom, P. M.; Chen, Yu-Jiuan; Poulsen, P.

    2001-06-01

    The typical response of the x-ray converter material to the passage of a high-powered relativistic electron beam is vaporization and rapid dispersal. The effect of this dispersal on subsequent pulses for multi-pulse radiography is the collective effects on the propagation of the electron beam through the expanding plasma and the reduced number of electron to photon interactions. Thus, for the dual-axis radiographic hydrodynamic test facility, the converter material must either be replaced or confined long enough to accommodate the entire pulse train. Typically the 1-mm-thick high Z and full density converter material is chosen to give peak dose and minimum radiographic spot. For repeated pulses we propose a modified converter, constructed of either low density, high Z material in the form of foam or of foils spaced over ten times the axial thickness of the standard 1 mm converter. The converter material is confined within a tube to impede outward motion in radius outside the beam interaction region. We report single-pulse experiments which measure the dose and spot size produced by the modified converter and compare them to similar measurements made by the standard converter. For multiple pulses over a microsecond time scale, we calculate the radial and axial hydrodynamic flow to study the material reflux into the converter volume and the resultant density decrease as the electron beam energy is deposited. Both the electron transport through the expanding low density plasma and beam in the higher density material are modeled. The x-ray source dose and spot size are calculated to evaluate the impact of the changing converter material density distribution on the radiographic spot size and dose. The results indicate that a multiple-pulse converter design for three or four high-power beam pulses is feasible.

  11. Shutterless ion mobility spectrometer with fast pulsed electron source

    Science.gov (United States)

    Bunert, E.; Heptner, A.; Reinecke, T.; Kirk, A. T.; Zimmermann, S.

    2017-02-01

    Ion mobility spectrometers (IMS) are devices for fast and very sensitive trace gas analysis. The measuring principle is based on an initial ionization process of the target analyte. Most IMS employ radioactive electron sources, such as 63Ni or 3H. These radioactive materials have the disadvantage of legal restrictions and the electron emission has a predetermined intensity and cannot be controlled or disabled. In this work, we replaced the 3H source of our IMS with 100 mm drift tube length with our nonradioactive electron source, which generates comparable spectra to the 3H source. An advantage of our emission current controlled nonradioactive electron source is that it can operate in a fast pulsed mode with high electron intensities. By optimizing the geometric parameters and developing fast control electronics, we can achieve very short electron emission pulses for ionization with high intensities and an adjustable pulse width of down to a few nanoseconds. This results in small ion packets at simultaneously high ion densities, which are subsequently separated in the drift tube. Normally, the required small ion packet is generated by a complex ion shutter mechanism. By omitting the additional reaction chamber, the ion packet can be generated directly at the beginning of the drift tube by our pulsed nonradioactive electron source with only slight reduction in resolving power. Thus, the complex and costly shutter mechanism and its electronics can also be omitted, which leads to a simple low-cost IMS-system with a pulsed nonradioactive electron source and a resolving power of 90.

  12. Pulsed Power for a Dynamic Transmission Electron Microscope

    Energy Technology Data Exchange (ETDEWEB)

    dehope, w j; browning, n; campbell, g; cook, e; king, w; lagrange, t; reed, b; stuart, b; Shuttlesworth, R; Pyke, B

    2009-06-25

    Lawrence Livermore National Laboratory (LLNL) has converted a commercial 200kV transmission electron microscope (TEM) into an ultrafast, nanoscale diagnostic tool for material science studies. The resulting Dynamic Transmission Electron Microscope (DTEM) has provided a unique tool for the study of material phase transitions, reaction front analyses, and other studies in the fields of chemistry, materials science, and biology. The TEM's thermionic electron emission source was replaced with a fast photocathode and a laser beam path was provided for ultraviolet surface illumination. The resulting photoelectron beam gives downstream images of 2 and 20 ns exposure times at 100 and 10 nm spatial resolution. A separate laser, used as a pump pulse, is used to heat, ignite, or shock samples while the photocathode electron pulses, carefully time-synchronized with the pump, function as probe in fast transient studies. The device functions in both imaging and diffraction modes. A laser upgrade is underway to make arbitrary cathode pulse trains of variable pulse width of 10-1000 ns. Along with a fast e-beam deflection scheme, a 'movie mode' capability will be added to this unique diagnostic tool. This talk will review conventional electron microscopy and its limitations, discuss the development and capabilities of DTEM, in particularly addressing the prime and pulsed power considerations in the design and fabrication of the DTEM, and conclude with the presentation of a deflector and solid-state pulser design for Movie-Mode DTEM.

  13. Free Electron Laser Pulse Control by Acousto Optic Modulators

    CERN Document Server

    Kanai, T; Yoshihashi-Suzuki, S

    2005-01-01

    Free Electron Laser (FEL) at Osaka University can be continuously varied in the range of 5.0-20.0 μm. A FEL has a double pulse structure. The structure consists of a train of macropulses of the pulse width 15 μs, and each macropulse contains a train of 330 micropulses of the pulse width 5 ps. The tunability and short pulse afford new medical applications such as investigation of protein dynamics and ablation of soft tissues. Precise control of micropulse train is very important for medical applications using FEL because macropulse with long pulse duration sometimes leads to undesirable thermal effects. FEL pulse control system using an acousto optic modulators (AOM) was developed in order to investigate of non-thermal effect between the FEL and tissue. This system provide a very good efficiency (~60 %) and a fast switching speed (>200 ns). A phosphorylated protein was irradiated with FEL that controlled the pulse. These result confirmed that the thermal effect is controlled by pulse durat...

  14. Attosecond physics at the nanoscale

    Czech Academy of Sciences Publication Activity Database

    Ciappina, Marcelo F.; Perez-Hernandez, J.A.; Landsman, A.S.; Okell, W.A.; Zherebtsov, S.; Foerg, B.; Schoetz, J.; Seiffert, L.; Fennel, T.; Shaaran, T.; Zimmermann, T.; Chacon, A.; Guichard, R.; Zair, A.; Tisch, J.W.G.; Marangos, J.P.; Witting, T.; Braun, A.; Maier, S. A.; Roso, L.; Krueger, M.; Hommelhoff, P.; Kling, M.F.; Krausz, F.; Lewenstein, M.

    2017-01-01

    Roč. 80, č. 5 (2017), 1-50, č. článku 054401. ISSN 0034-4885 R&D Projects: GA MŠk EF15_008/0000162; GA MŠk LQ1606 Grant - others:ELI Beamlines(XE) CZ.02.1.01/0.0/0.0/15_008/0000162 Institutional support: RVO:68378271 Keywords : attosecond physics * plasmonic fields * strong field physics Subject RIV: BH - Optics, Masers, Lasers Impact factor: 14.311, year: 2016

  15. Temporary acceleration of electrons while inside an intense electromagnetic pulse

    Directory of Open Access Journals (Sweden)

    Kirk T. McDonald

    1999-12-01

    Full Text Available A free electron can temporarily gain a very significant amount of energy if it is overrun by an intense electromagnetic wave. In principle, this process would permit large enhancements in the center-of-mass energy of electron-electron, electron-positron, and electron-photon interactions if these take place in the presence of an intense laser beam. Practical considerations severely limit the utility of this concept for contemporary lasers incident on relativistic electrons. A more accessible laboratory phenomenon is electron-positron production via an intense laser beam incident on a gas. Intense electromagnetic pulses of astrophysical origin can lead to very energetic photons via bremsstrahlung of temporarily accelerated electrons.

  16. Nonlinear electron emission in ultrashort laser pulses and rescattering suppression

    Science.gov (United States)

    Mikhin, E. A.; Preobrazhenskii, M. A.; Golovinski, P. A.

    2017-11-01

    The process of nonlinear electron emission from a metal surface under the action of femtosecond laser pulse with moderate intensity ~1011 W/cm2 is considered. One-dimensional model is formulated, taking into account the advantage of the p-polarized light in the nonlinear emission. The time dependent Schrödinger equation with fixed equilibrium boundary conditions is solved in the half-space using the Laplace transform technique. The energy spectrum of emitted electrons is presented, including analysis of dependence on the laser pulse parameters. In the framework of classical mechanics, the impact of additional dc electric field on the rescattering of emitted electron on the metal surface is investigated. The model reproduces the fiches of electron energy distribution and can be used at arbitrary Keldysh parameters.

  17. Ultrashort laser pulse driven inverse free electron laser accelerator experiment

    Directory of Open Access Journals (Sweden)

    J. T. Moody

    2016-02-01

    Full Text Available In this paper we discuss the ultrashort pulse high gradient inverse free electron laser accelerator experiment carried out at the Lawrence Livermore National Laboratory which demonstrated gradients exceeding 200  MV/m using a 4 TW 100 fs long 800 nm Ti:Sa laser pulse. Due to the short laser and electron pulse lengths, synchronization was determined to be one of the main challenges in this experiment. This made necessary the implementation of a single-shot, nondestructive, electro-optic sampling based diagnostics to enable time-stamping of each laser accelerator shot with <100  fs accuracy. The results of this experiment are expected to pave the way towards the development of future GeV-class IFEL accelerators.

  18. First-principles electron dynamics control simulation of diamond under femtosecond laser pulse train irradiation.

    Science.gov (United States)

    Wang, Cong; Jiang, Lan; Wang, Feng; Li, Xin; Yuan, Yanping; Xiao, Hai; Tsai, Hai-Lung; Lu, Yongfeng

    2012-07-11

    A real-time and real-space time-dependent density functional is applied to simulate the nonlinear electron-photon interactions during shaped femtosecond laser pulse train ablation of diamond. Effects of the key pulse train parameters such as the pulse separation, spatial/temporal pulse energy distribution and pulse number per train on the electron excitation and energy absorption are discussed. The calculations show that photon-electron interactions and transient localized electron dynamics can be controlled including photon absorption, electron excitation, electron density, and free electron distribution by the ultrafast laser pulse train.

  19. Desorption by Femtosecond Laser Pulses : An Electron-Hole Effect?

    OpenAIRE

    D. M., NEWNS; T. F., HEINZ; J. A., MISEWICH; IBM Research Division, T. J. Watson Research Center; IBM Research Division, T. J. Watson Research Center; IBM Research Division, T. J. Watson Research Center

    1992-01-01

    Desorption of molecules from metal surfaces induced by femtosecond visible laser pulses has been reported. Since the lattice temperature rise is insufficient to explain desorption, an electronic mechanism is clearly responsible. It is shown that a theory based on direct coupling between the center-of-mass degree of freedom of the adsorbate and the electron-hole excitations of the substrate provides a satisfactory explanation of the various experimental findings.

  20. Autocorrelation measurement of fast electron pulses emitted through the interaction of femtosecond laser pulses with a solid target.

    Science.gov (United States)

    Inoue, Shunsuke; Tokita, Shigeki; Otani, Kazuto; Hashida, Masaki; Hata, Masayasu; Sakagami, Hitoshi; Taguchi, Toshihiro; Sakabe, Shuji

    2012-11-02

    We report the first direct measurement of the emission duration of laser-accelerated fast electrons from the surface of a solid target irradiated by a high-intensity femtosecond laser pulse. The emission duration is determined by autocorrelation measurement using the Coulomb repulsive forces that act on two equivalent electron pulses. The emission duration depends on the laser pulse duration for laser pulses of 200-690 fs. Numerical modeling of three-dimensional charged particle dynamics indicates that the emission duration of fast electrons is almost equal to the duration of the laser pulse.

  1. Short electron bunches generated by perpendicularly crossing laser pulses

    Science.gov (United States)

    Horný, Vojtěch; Petržílka, Václav; Klimo, Ondřej; Krůs, Miroslav

    2017-10-01

    Optical injection of electrons into a laser wakefield accelerator by a low intensity orthogonally colliding laser pulse is investigated using 2D particle-in-cell simulations. The collision of the main laser pulse driving the plasma wave in the cavitated regime and the low intensity injection pulse affects the trajectories of electrons in the crossing region. As a consequence, some electrons are ejected into the front part of the bubble, and these electrons are subsequently trapped in the rear part of the bubble. The injected and accelerated electron bunch reaches a peak energy of 630 MeV after 8 ps of acceleration being as short as 7.0 fs and is quasimonoenergetic with a low energy spread of 20 MeV (3.8%), having a charge of several dozens of pC and a relatively large emittance of 2.27 π . mm . mrad. Two main injection mechanisms—crossing beatwave injection and injection by laser field preacceleration—were identified.

  2. High current precision long pulse electron beam position monitor

    CERN Document Server

    Nelson, S D; Fessenden, T J; Holmes, C

    2000-01-01

    Precision high current long pulse electron beam position monitoring has typically experienced problems with high Q sensors, sensors damped to the point of lack of precision, or sensors that interact substantially with any beam halo thus obscuring the desired signal. As part of the effort to develop a multi-axis electron beam transport system using transverse electromagnetic stripline kicker technology, it is necessary to precisely determine the position and extent of long high energy beams for accurate beam position control (6 - 40 MeV, 1 - 4 kA, 2 μs beam pulse, sub millimeter beam position accuracy.) The kicker positioning system utilizes shot-to-shot adjustments for reduction of relatively slow (< 20 MHz) motion of the beam centroid. The electron beams passing through the diagnostic systems have the potential for large halo effects that tend to corrupt position measurements.

  3. Investigating Pulsed Discharge Polarity Employing Solid-State Pulsed Power Electronics

    DEFF Research Database (Denmark)

    Davari, Pooya; Zare, Firuz; Blaabjerg, Frede

    2015-01-01

    Power electronics technique has become a key technology in solid-state pulsed power supplies. Since pulsed power applications have been matured and found its way into many industrial applications, moving toward energy efficiency is gaining much more interest. Therefore, finding an optimum operation......, the influence of electric field distribution is analyzed using Finite Element simulations for the employed geometries and mediums. The experimental and simulation results have verified the important role of the applied voltage polarity, employed geometry and medium of the system on plasma generation....

  4. Anterior capsulotomy with a pulsed-electron avalanche knife.

    Science.gov (United States)

    Palanker, Daniel; Nomoto, Hiroyuki; Huie, Philip; Vankov, Alexander; Chang, David F

    2010-01-01

    To evaluate a new pulsed-electron avalanche knife design for creating a continuous curvilinear capsulotomy (CCC) and compare the CCC with a mechanical capsulorhexis. Department of Ophthalmology, Stanford University, Stanford, California, USA. In this study, CCCs were created in freshly enucleated bovine eyes and in rabbit eyes in vivo. The cutting velocity was adjusted by controlling the burst repetition rate, voltage amplitude, and burst duration. Tissue samples were fixed and processed for histology and scanning electron microscopy (SEM) immediately after surgery. The study included 50 bovine eyes and 10 rabbit eyes. By adjusting the electrosurgical waveforms, gas-bubble formation was minimized to permit good surgical visualization. The optimum voltage level was determined to be +/-410 V with a burst duration of 20 mus. Burst repetition rate, continuously adjustable from 20 to 200 Hz with footpedal control, allowed the surgeon to vary linear cutting velocity up to 2.0 mm/s. Histology and SEM showed that the pulsed-electron avalanche knife produced sharp-edged capsule cutting without radial nicks or tears. The probe of the pulsed-electron avalanche knife duplicated the surgical feel of a 25-gauge cystotome and created a histologically smooth capsule cut. It may improve precision and reproducibility of creating a CCC, as well as improve its proper sizing and centration, especially in the face of surgical risk factors, such as weak zonules or poor visibility. Drs. Palanker and Vankov hold patents to the pulsed electron avalanche knife technology, which are licensed to PEAK Surgical by Stanford University. Drs. Palanker and Chang are consultants to PEAK Surgical. Dr. Vankov is an employee of PEAK Surgical. Neither of the other authors has a financial or proprietary interest in any material or method mentioned. Copyright 2010 ASCRS and ESCRS. Published by Elsevier Inc. All rights reserved.

  5. Electron pulse shaping in the FELIX RF accelerator

    CERN Document Server

    Weits, H H; Oepts, D; Van der Meer, Alex F G

    1999-01-01

    The FELIX free-electron laser uses short pulses of relativistic electrons produced by an RF accelerator. The design target for the duration of these electron bunches was around 3 ps. In experiments we observed that the bunches emit coherently enhanced spontaneous emission (CSE) when they travel through an undulator. It was demonstrated that the power level of the CSE critically depends on the settings of the accelerator. In this article we seek to explain these observations by studying the length and shape of the electron bunches as a function of the settings of the accelerator. A particle- tracking model was used to simulate the acceleration and transport processes. These include bunch compression in a 14-cell travelling wave buncher cavity, acceleration in a travelling wave linear accelerator, and passage through a (dispersive) chicane structure. The effect of the phase setting of the RF accelerating field with respect to the arrival time of the electron bunch in each accelerator structure was studied. The ...

  6. Plasma high-order-harmonic generation from ultraintense laser pulses

    Science.gov (United States)

    Tang, Suo; Kumar, Naveen; Keitel, Christoph H.

    2017-05-01

    Plasma high-order-harmonic generation from an extremely intense short-pulse laser is explored by including the effects of ion motion, electron-ion collisions, and radiation reaction force in the plasma dynamics. The laser radiation pressure induces plasma ion motion through the hole-boring effect, resulting in frequency shifting and widening of the harmonic spectra. The classical radiation reaction force slightly mitigates the frequency broadening caused by the ion motion. Based on the results and physical considerations, parameter maps highlighting the optimum regions for generating a single intense attosecond pulse and coherent XUV radiation are presented.

  7. Femtosecond single-electron diffraction.

    Science.gov (United States)

    Lahme, S; Kealhofer, C; Krausz, F; Baum, P

    2014-05-01

    Ultrafast electron diffraction allows the tracking of atomic motion in real time, but space charge effects within dense electron packets are a problem for temporal resolution. Here, we report on time-resolved pump-probe diffraction using femtosecond single-electron pulses that are free from intra-pulse Coulomb interactions over the entire trajectory from the source to the detector. Sufficient average electron current is achieved at repetition rates of hundreds of kHz. Thermal load on the sample is avoided by minimizing the pump-probe area and by maximizing heat diffusion. Time-resolved diffraction from fibrous graphite polycrystals reveals coherent acoustic phonons in a nanometer-thick grain ensemble with a signal-to-noise level comparable to conventional multi-electron experiments. These results demonstrate the feasibility of pump-probe diffraction in the single-electron regime, where simulations indicate compressibility of the pulses down to few-femtosecond and attosecond duration.

  8. Femtosecond single-electron diffraction

    Directory of Open Access Journals (Sweden)

    S. Lahme

    2014-05-01

    Full Text Available Ultrafast electron diffraction allows the tracking of atomic motion in real time, but space charge effects within dense electron packets are a problem for temporal resolution. Here, we report on time-resolved pump-probe diffraction using femtosecond single-electron pulses that are free from intra-pulse Coulomb interactions over the entire trajectory from the source to the detector. Sufficient average electron current is achieved at repetition rates of hundreds of kHz. Thermal load on the sample is avoided by minimizing the pump-probe area and by maximizing heat diffusion. Time-resolved diffraction from fibrous graphite polycrystals reveals coherent acoustic phonons in a nanometer-thick grain ensemble with a signal-to-noise level comparable to conventional multi-electron experiments. These results demonstrate the feasibility of pump-probe diffraction in the single-electron regime, where simulations indicate compressibility of the pulses down to few-femtosecond and attosecond duration.

  9. Ultrashort X-ray pulse generation using subpicosecond electron linac

    CERN Document Server

    Harano, H; Yoshii, K; Ueda, T; Okita, S; Uesaka, M

    2000-01-01

    As a promising tool for ultrafast material analyses, we propose to utilize the X-ray pulse which may be generated in a quite simple manner using subpicosecond electron linacs. The properties of the X-ray were numerically studied with the EGS4 code. Verification of the X-ray generation was also conducted at the Nuclear Engineering Research Laboratory (NERL) linac and clear diffraction patterns of characteristic X-ray were obtained for typical single crystals.

  10. High-power 95 GHz pulsed electron spin resonance spectrometer

    Science.gov (United States)

    Hofbauer, W.; Earle, K. A.; Dunnam, C. R.; Moscicki, J. K.; Freed, J. H.

    2004-05-01

    High-field/high-frequency electron spin resonance (ESR) offers improved sensitivity and resolution compared to ESR at conventional fields and frequencies. However, most high-field/high-frequency ESR spectrometers suffer from limited mm-wave power, thereby requiring long mm-wave pulses. This precludes their use when relaxation times are short, e.g., in fluid samples. Low mm-wave power is also a major factor limiting the achievable spectral coverage and thereby the multiplex advantage of Fourier transform ESR (FTESR) experiments. High-power pulses are needed to perform two-dimensional (2D) FTESR experiments, which can unravel the dynamics of a spin system in great detail, making it an excellent tool for studying spin and molecular dynamics. We report on the design and implementation of a high-power, high-bandwidth, pulsed ESR spectrometer operating at 95 GHz. One of the principal design goals was the ability to investigate dynamic processes in aqueous samples at physiological temperatures with the intent to study biological systems. In initial experiments on aqueous samples at room temperature, we achieved 200 MHz spectral coverage at a sensitivity of 1.1×1010√s spins and a dead time of less than 50 ns. 2D-electron-electron double resonance experiments on aqueous samples are discussed to demonstrate the practical application of such a spectrometer.

  11. Non-linear electron photoemission from metals with ultrashort pulses

    Energy Technology Data Exchange (ETDEWEB)

    Ferrini, Gabriele; Banfi, Francesco; Giannetti, Claudio [Dipartimento di Matematica e Fisica, Universita Cattolica del Sacro Cuore, I-25121 Brescia (Italy); Parmigiani, Fulvio [Dipartimento di Fisica, Universita di Trieste and Sincrotrone Trieste, Strada Statale 14, I-34012 Basovizza, Trieste (Italy)], E-mail: fulvio.parmigiani@elettra.trieste.it

    2009-03-21

    In this review we describe the development of ultrafast non-linear photoemission spectroscopy on metals from the first historic observations in the sixties to state-of-the-art experiments. We present an account that is focused on electron spectroscopy experiments that use short laser pulses to investigate the non-equilibrium response of electrons in metals. Several examples of the application of non-linear spectroscopy to the investigation of many-body effects and highly non-equilibrium processes will be illustrated. Furthermore, we give a brief overview of the wide spectrum of experimental methods based on non-linear photoemission spectroscopy.

  12. Modelling hot electron generation in short pulse target heating experiments

    Directory of Open Access Journals (Sweden)

    Sircombe N.J.

    2013-11-01

    Full Text Available Target heating experiments planned for the Orion laser facility, and electron beam driven fast ignition schemes, rely on the interaction of a short pulse high intensity laser with dense material to generate a flux of energetic electrons. It is essential that the characteristics of this electron source are well known in order to inform transport models in radiation hydrodynamics codes and allow effective evaluation of experimental results and forward modelling of future campaigns. We present results obtained with the particle in cell (PIC code EPOCH for realistic target and laser parameters, including first and second harmonic light. The hot electron distributions are characterised and their implications for onward transport and target heating are considered with the aid of the Monte-Carlo transport code THOR.

  13. Electron optical injection with head-on and countercrossing colliding laser pulses.

    Science.gov (United States)

    Kotaki, H; Daito, I; Kando, M; Hayashi, Y; Kawase, K; Kameshima, T; Fukuda, Y; Homma, T; Ma, J; Chen, L-M; Esirkepov, T Zh; Pirozhkov, A S; Koga, J K; Faenov, A; Pikuz, T; Kiriyama, H; Okada, H; Shimomura, T; Nakai, Y; Tanoue, M; Sasao, H; Wakai, D; Matsuura, H; Kondo, S; Kanazawa, S; Sugiyama, A; Daido, H; Bulanov, S V

    2009-11-06

    A high stability electron bunch is generated by laser wakefield acceleration with the help of a colliding laser pulse. The wakefield is generated by a laser pulse; the second laser pulse collides with the first pulse at 180 degrees and at 135 degrees realizing optical injection of an electron bunch. The electron bunch has high stability and high reproducibility compared with single pulse electron generation. In the case of 180 degrees collision, special measures have been taken to prevent damage. In the case of 135 degrees collision, since the second pulse is countercrossing, it cannot damage the laser system.

  14. Attosecond interference in strong-field nonsequential double ionization

    Science.gov (United States)

    Liao, Qing; Li, Ye; Qin, Meiyan; Lu, Peixiang

    2017-12-01

    Kinetic-energy spectra of a single electron from strong-field nonsequential double ionization are investigated in a high-intensity regime with a quantum mechanical model. We find interference fringes with large energy spacings, which increases with the electron kinetic energy. These interference fringes originate from the electronic wave packets born in the recollision by the returning electronic wave packets from the "short" and the "long" quantum paths. Since the recollision happens in a fraction of a near-infrared (NIR) optical cycle, i.e., in an attosecond time interval, the resulting interference fringes exhibit energy spacings much larger than the NIR photon energy. The comparison of the quantum mechanical results with a classical collision model suggests a near-equal energy sharing between two electrons during the recollision process at very high intensities, in contrast to the extremely unequal energy sharing at low intensities.

  15. Silicon nanowire based high brightness, pulsed relativistic electron source

    Directory of Open Access Journals (Sweden)

    Deep Sarkar

    2017-06-01

    Full Text Available We demonstrate that silicon nanowire arrays efficiently emit relativistic electron pulses under irradiation by a high-intensity, femtosecond, and near-infrared laser (∼1018 W/cm2, 25 fs, 800 nm. The nanowire array yields fluxes and charge per bunch that are 40 times higher than those emitted by an optically flat surface, in the energy range of 0.2–0.5 MeV. The flux and charge yields for the nanowires are observed to be directional in nature unlike that for planar silicon. Particle-in-cell simulations establish that such large emission is caused by the enhancement of the local electric fields around a nanowire, which consequently leads to an enhanced absorption of laser energy. We show that the high-intensity contrast (ratio of picosecond pedestal to femtosecond peak of the laser pulse (10−9 is crucial to this large yield. We extend the notion of surface local-field enhancement, normally invoked in low-order nonlinear optical processes like second harmonic generation, optical limiting, etc., to ultrahigh laser intensities. These electron pulses, expectedly femtosecond in duration, have potential application in imaging, material modification, ultrafast dynamics, terahertz generation, and fast ion sources.

  16. Helicity-Selective Enhancement and Polarization Control of Attosecond High Harmonic Waveforms Driven by Bichromatic Circularly Polarized Laser Fields

    Science.gov (United States)

    Dorney, Kevin M.; Ellis, Jennifer L.; Hernández-García, Carlos; Hickstein, Daniel D.; Mancuso, Christopher A.; Brooks, Nathan; Fan, Tingting; Fan, Guangyu; Zusin, Dmitriy; Gentry, Christian; Grychtol, Patrik; Kapteyn, Henry C.; Murnane, Margaret M.

    2017-08-01

    High harmonics driven by two-color counterrotating circularly polarized laser fields are a unique source of bright, circularly polarized, extreme ultraviolet, and soft x-ray beams, where the individual harmonics themselves are completely circularly polarized. Here, we demonstrate the ability to preferentially select either the right or left circularly polarized harmonics simply by adjusting the relative intensity ratio of the bichromatic circularly polarized driving laser field. In the frequency domain, this significantly enhances the harmonic orders that rotate in the same direction as the higher-intensity driving laser. In the time domain, this helicity-dependent enhancement corresponds to control over the polarization of the resulting attosecond waveforms. This helicity control enables the generation of circularly polarized high harmonics with a user-defined polarization of the underlying attosecond bursts. In the future, this technique should allow for the production of bright highly elliptical harmonic supercontinua as well as the generation of isolated elliptically polarized attosecond pulses.

  17. Benchmarking Attosecond Physics with Atomic Hydrogen

    Science.gov (United States)

    2015-05-25

    Final 3. DATES COVERED (From - To) 12 Mar 12 – 11 Mar 15 4. TITLE AND SUBTITLE Benchmarking attosecond physics with atomic hydrogen 5a...AND SUBTITLE Benchmarking attosecond physics with atomic hydrogen 5a. CONTRACT NUMBER FA2386-12-1-4025 5b. GRANT NUMBER 5c. PROGRAM ELEMENT NUMBER...THIS PAGE unclassified Standard Form 298 (Rev. 8-98) Prescribed by ANSI Std Z39-18 Final Report for AOARD Grant FA2386-12-1-4025 “ Benchmarking

  18. Towards Attosecond High-Energy Electron Bunches: Controlling Self-Injection in Laser-Wakefield Accelerators Through Plasma-Density Modulation

    Science.gov (United States)

    Tooley, M. P.; Ersfeld, B.; Yoffe, S. R.; Noble, A.; Brunetti, E.; Sheng, Z. M.; Islam, M. R.; Jaroszynski, D. A.

    2017-07-01

    Self-injection in a laser-plasma wakefield accelerator is usually achieved by increasing the laser intensity until the threshold for injection is exceeded. Alternatively, the velocity of the bubble accelerating structure can be controlled using plasma density ramps, reducing the electron velocity required for injection. We present a model describing self-injection in the short-bunch regime for arbitrary changes in the plasma density. We derive the threshold condition for injection due to a plasma density gradient, which is confirmed using particle-in-cell simulations that demonstrate injection of subfemtosecond bunches. It is shown that the bunch charge, bunch length, and separation of bunches in a bunch train can be controlled by tailoring the plasma density profile.

  19. An Electronic Patch for Wearable Health Monitoring by Reflectance Pulse Oximetry

    DEFF Research Database (Denmark)

    Haahr, Rasmus Grønbek; Duun, Sune Bro; Toft, Mette H.

    2012-01-01

    . In this paper the Electronic Patch is demonstrated with a new optical biomedical sensor for reflectance pulse oximetry so that the Electronic Patch in this case can measure the pulse and the oxygen saturation. The reflectance pulse oximetry solution is based on a recently developed annular backside silicon...

  20. Single-cycle Optical Pulses and Isolated Attosecond Pulse Generation

    Science.gov (United States)

    2012-02-29

    picosecond green light from a frequency-doubled hybrid cryogenic Yb:YAG laser system,” 36 UFO /HFSW 2009 (Arcachon, France, Aug. 31-Sept. 4, 2009...High Fields Short Wavelength,” ( UFO VII – HFSW XIII), Arcachon, France, August 31 – September 4, 2009 (invited). 25) Kyung-Han Hong, Juliet Gopinath

  1. Pulsed electron avalanche knife (PEAK) for intraocular surgery.

    Science.gov (United States)

    Palanker, D V; Miller, J M; Marmor, M F; Sanislo, S R; Huie, P; Blumenkranz, M S

    2001-10-01

    To develop a better and more economical instrument for precise, tractionless, "cold" cutting during intraocular surgery. The use of highly localized electric fields rather than laser light as the means of tissue dissection was investigated. A high electric field at the tip of a fine wire can, like lasers, initiate plasma formation. Micrometer-length plasma streamers are generated when an insulated 25 micron (microm) wire, exposed to physiological medium at one end, is subjected to nanosecond electrical pulses between 1 and 8 kV in magnitude. The explosive evaporation of water in the vicinity of these streamers cuts soft tissue without heat deposition into surrounding material (cold cutting). Streamers of plasma and the dynamics of water evaporation were imaged using an inverted microscope and fast flash photography. Cutting effectiveness was evaluated on both polyacrylamide gels, on different tissues from excised bovine eyes, and in vivo on rabbit retina. Standard histology techniques were used to examine the tissue. Electric pulses with energies between 150 and 670 microJ produced plasma streamers in saline between 10 and 200 microm in length. Application of electric discharges to dense (10%) polyacrylamide gels resulted in fracturing of the gel without ejection of bulk material. In both dense and softer (6%) gels, layer by layer shaving was possible with pulse energy rather than number of pulses as the determinant of ultimate cutting depth. The instrument made precise partial or full-thickness cuts of retina, iris, lens, and lens capsule without any evidence of thermal damage. Because different tissues require distinct energies for dissection, tissue-selective cutting on complex structures can be performed if the appropriate pulse energies are used; for example, retina can be dissected without damage to the major retinal vessels. This instrument, called the Pulsed Electron Avalanche Knife (PEAK), can quickly and precisely cut intraocular tissues without traction

  2. Quantum path interferences of electron trajectories in two-center molecules.

    Science.gov (United States)

    Yang, Weifeng; Song, Xiaohong; Zeng, Zhinan; Li, Ruxin; Xu, Zhizhan

    2010-02-01

    We report a new quantum path interference effect of electron trajectories in high-order harmonic generation (HHG) from two-center molecules, in which the interference minima are mainly located in the high-energy portion of HHG spectrum. The quantum calculations of the time-frequency analyses and the classical results of the electron trajectories demonstrate very good agreement and reveal that the positions of the interference minima are associated with the cutoff of various kinds of molecular electron trajectories. The interference fringes within a half optical cycle can be clearly seen in the time-frequency analysis spectrum. Moreover, the characteristics of both the HHG in frequency domain and the corresponding attosecond pulse generation in time domain permit tracing back the interference information of these electron trajectories. These interference phenomena offer new possibilities for getting insight into the attosecond electronic dynamics in molecules.

  3. Pulsed electron beam annealing of As and B implanted silicon

    Energy Technology Data Exchange (ETDEWEB)

    Barbier, D.; Chemisky, G.; Laugier, A. (Institut National des Sciences Appliquees de Lyon 69 - Villeurbanne (France)); Grob, J.J.; Siffert, P.; Stuck, R. (Centre de Recherche Nucleaire, 67 - Strasbourg (France))

    1983-01-01

    p-type (100) silicon wafers have been implanted either by As or B ions at 20 and 200 keV energies and doses of 10/sup 16/cm/sup -2/. Pulsed electron beam annealing has been performed with fluences of 1.1 and 1.4J/cm/sup 2/ using a mean electron energy of 15 keV. The pulse duration was 50 ns. The annealed layers have been investigated by Rutherford backscattering under random and channeling conditions and by S.I.M.S. profiling. Good crystal regrowth and high dopant activation occur in all cases except for the 200 keV Boron implant. Impurities redistribution is observed but no significant segregation effects appear. The experimental profiles are in good agreement with a diffusion model using a modified green function solution and taking into account dopant diffusion in liquid phase and the computed melt front location. The deduced diffusion coefficient are in the 5.10/sup -5/cm/sup 2//s range for boron and 2.10/sup -4/cm/sup 2//s range for arsenic.

  4. Deconfinement of Quarks with TeV Attosecond Photon Beams

    Science.gov (United States)

    Stefan, V. Alexander

    2010-02-01

    Recently, I have proposed a novel heuristic method for the deconfinement of quarks.footnotetextM. Gell-Mann. The Quark and the Jaguar: Adventures in the Simple and the Complex (New York, NY: W.H. Freeman and Co., 1994) [cf. M. Gell-Mann, The Garden of Live Flowers in: V. Stefan (Editor), Physics and Society. Essays Honoring Victor Frederick Weisskopf (Springer, 1998), pp. 109-121]. It proceeds in two phases.footnotetextV. Alexander Stefan, On a Heuristic Point of View About Inertial Deconfinement of Quarks, American Physical Society, 2009 APS April Meeting, May 2-5, 2009, abstract #E1.038. Firstly, a frozen hydrogen pellet is inertially confined by the ultra-intense lasers up to a solid state density. Secondly, a solid state nano-pellet is ``punched'' by the photon beam created in the beat wave driven free electron laser (BW-FEL), leading to the ``rapture'' (in a ``karate chop'' model) of the ``MIT Bag''footnotetextJ. I. Friedman and H. Kendall, Viki, in: V. Stefan (Editor), Physics and Society. (Springer, 1998), pp. 103-108]. before the asymptotically free quarks move apart. Hereby, I propose TeV, a few 100s attosecond, photon beams in interaction with the nano-pellet. The threshold ``rapture force'' of the TeV attosecond photon is 10^7 N. )

  5. Two electron response to an intense x-ray free electron laser pulse

    Energy Technology Data Exchange (ETDEWEB)

    Moore, L R; Parker, J S; Meharg, K J; Armstrong, G S J; Taylor, K T, E-mail: l.moore@qub.ac.u [DAMTP, David Bates Building, Queen' s University Belfast, Belfast, BT7 1NN (United Kingdom)

    2009-11-01

    New x-ray free electron lasers (FELs) promise an ultra-fast ultra-intense regime in which new physical phenomena, such as double core hole formation in at atom, should become directly observable. Ahead of x-ray FEL experiments, an initial key task is to theoretically explore such fundamental laser-atom interactions and processes. To study the response of a two-electron positive ion to an intense x-ray FEL pulse, our theoretical approach is a direct numerical integration, incorporating non-dipole Hamiltonian terms, of the full six-dimensional time-dependent Schroedinger equation. We present probabilities of double K-shell ionization in the two-electron positive ions Ne{sup 8+} and Ar{sup 16+} exposed to x-ray FEL pulses with frequencies in the range 50 au to 300 au and intensities in the range 10{sup 17} to 10{sup 22} W/cm{sup 2}.

  6. Design and implementation of an FPGA-based timing pulse programmer for pulsed-electron paramagnetic resonance applications.

    Science.gov (United States)

    Sun, Li; Savory, Joshua J; Warncke, Kurt

    2013-08-01

    The design, construction and implementation of a field-programmable gate array (FPGA) -based pulse programmer for pulsed-electron paramagnetic resonance (EPR) experiments is described. The FPGA pulse programmer offers advantages in design flexibility and cost over previous pulse programmers, that are based on commercial digital delay generators, logic pattern generators, and application-specific integrated circuit (ASIC) designs. The FPGA pulse progammer features a novel transition-based algorithm and command protocol, that is optimized for the timing structure required for most pulsed magnetic resonance experiments. The algorithm was implemented by using a Spartan-6 FPGA (Xilinx), which provides an easily accessible and cost effective solution for FPGA interfacing. An auxiliary board was designed for the FPGA-instrument interface, which buffers the FPGA outputs for increased power consumption and capacitive load requirements. Device specifications include: Nanosecond pulse formation (transition edge rise/fall times, ≤3 ns), low jitter (≤150 ps), large number of channels (16 implemented; 48 available), and long pulse duration (no limit). The hardware and software for the device were designed for facile reconfiguration to match user experimental requirements and constraints. Operation of the device is demonstrated and benchmarked by applications to 1-D electron spin echo envelope modulation (ESEEM) and 2-D hyperfine sublevel correlation (HYSCORE) experiments. The FPGA approach is transferrable to applications in nuclear magnetic resonance (NMR; magnetic resonance imaging, MRI), and to pulse perturbation and detection bandwidths in spectroscopies up through the optical range.

  7. A laser triggered electron source for pulsed radiolysis

    CERN Document Server

    Monard, H; Le Duff, J; Garvey, Terence; Mouton, B; Rodier, J; Thiery, Y; Gaillard, M

    1999-01-01

    We present the design of a photo-injector based accelerator for pulsed radiolysis applications. This machine is destined to meet the needs of the physical chemistry community at the Universite de Paris XI. A 4 MeV Energy electron pulse of a few picoseconds duration and with a charge in the range of 1 to 10 nC is produced from a Cs/sub 2 /Te photocathode. The photocathode is placed in the half energy spread cell of a 1-1/2 cell, 3 GHz RF gun, whose design is based on the gun used for the drive beam of the CERN CLIC Test facility. A 4 cell "booster" cavity is then used to accelerate the beam to an energy of 9 MeV. The transport system consists of a quadrupole triplet downsteam of the booster, two rectangular, 30 degree bend, dipoles with a pair of quadrupoles between them and a second triplet downstream of the second dipole. Energy dependent path length effects in the two dipoles allow the possibility of magnetic bunch compression depending on the phase-energy correlation of the bunch exiting the booster cavity...

  8. Optimization and control of electron beams from laser wakefield accelerations using asymmetric laser pulses

    Science.gov (United States)

    Gopal, K.; Gupta, D. N.

    2017-10-01

    Optimization and control of electron beam quality in laser wakefield acceleration are explored by using a temporally asymmetric laser pulse of the sharp rising front portion. The temporally asymmetric laser pulse imparts stronger ponderomotive force on the ambient plasma electrons. The stronger ponderomotive force associated with the asymmetric pulse significantly affects the injection of electrons into the wakefield and consequently the quality of the injected bunch in terms of injected charge, mean energy, and emittance. Based on particle-in-cell simulations, we report to generate a monoenergetic electron beam with reduced emittance and enhanced charge in laser wakefield acceleration using an asymmetric pulse of duration 30 fs.

  9. Externally Controlled Injection of Electrons by a Laser Pulse in a Laser Wakefield Electron Accelerator

    CERN Document Server

    Chen Szu Yuan; Chen Wei Ting; Chien, Ting-Yei; Lee, Chau-Hwang; Lin, Jiunn-Yuan; Wang, Jyhpyng

    2005-01-01

    Spatially and temporally localized injection of electrons is a key element for development of plasma-wave electron accelerator. Here we report the demonstration of two different schemes for electron injection in a self-modulated laser wakefield accelerator (SM-LWFA) by using a laser pulse. In the first scheme, by implementing a copropagating laser prepulse with proper timing, we are able to control the growth of Raman forward scattering and the production of accelerated electrons. We found that the stimulated Raman backward scattering of the prepulse plays the essential role of injecting hot electrons into the fast plasma wave driven by the pump pulse. In the second scheme, by using a transient density ramp we achieve self-injection of electrons in a SM-LWFA with spatial localization. The transient density ramp is produced by a prepulse propagating transversely to drill a density depression channel via ionization and expansion. The same mechanism of injection with comparable efficiency is also demonstrated wi...

  10. Constraints on photon pulse duration from longitudinal electron beam diagnostics at a soft x-ray free-electron laser

    Directory of Open Access Journals (Sweden)

    C. Behrens

    2012-03-01

    Full Text Available The successful operation of x-ray free-electron lasers (FELs, like the Linac Coherent Light Source or the Free-Electron Laser in Hamburg (FLASH, makes unprecedented research on matter at atomic length and ultrafast time scales possible. However, in order to take advantage of these unique light sources and to meet the strict requirements of many experiments in photon science, FEL photon pulse durations need to be known and tunable. This can be achieved by controlling the FEL driving electron beams, and high-resolution longitudinal electron beam diagnostics can be utilized to provide constraints on the expected FEL photon pulse durations. In this paper, we present comparative measurements of soft x-ray pulse durations and electron bunch lengths at FLASH. The soft x-ray pulse durations were measured by FEL radiation pulse energy statistics and compared to electron bunch lengths determined by frequency-domain spectroscopy of coherent transition radiation in the terahertz range and time-domain longitudinal phase space measurements. The experimental results, theoretical considerations, and simulations show that high-resolution longitudinal electron beam diagnostics provide reasonable constraints on the expected FEL photon pulse durations. In addition, we demonstrated the generation of soft x-ray pulses with durations below 50 fs (FWHM after the implementation of the new uniform electron bunch compression scheme used at FLASH.

  11. Multiscale dynamics of C60 from attosecond to statistical physics

    Science.gov (United States)

    Lépine, F.

    2015-06-01

    C60 is a fascinating object that has become remarkably useful for experimentalists and theoreticians to study photo-induced processes in large many-particle systems. In this review article, we discuss how the knowledge accumulated over the past 30 years on this molecule provides a large panel of mechanisms that occur from the intrinsic time scale of electronic motion that is attosecond, to long ‘macroscopic’ time scale (second). This illustrates the multiscale aspect of dynamics in photo-excited systems, which connects coherent quantum processes to classical and statistical mechanisms. This also shines light onto future experiments and theoretical work required to complete the global picture of light-induced mechanisms in fullerenes.

  12. Pulse height measurements and electron attachment in drift chambers operated with Xe,CO2 mixtures

    CERN Document Server

    Andronic, A

    2003-01-01

    We present pulse height measurements in drift chambers operated with Xe,CO2 gas mixtures. We investigate the attachment of primary electrons on oxygen and SF6 contaminants in the detection gas. The measurements are compared with simulations of properties of drifting electrons. We present two methods to check the gas quality: gas chromatography and Fe55 pulse height measurements using monitor detectors.

  13. PERCEPTION LEVEL EVALUATION OF RADIO ELECTRONIC MEANS TO A PULSE OF ELECTROMAGNETIC RADIATION

    Directory of Open Access Journals (Sweden)

    2016-01-01

    Full Text Available The method for evaluating the perception level of electronic means to pulsed electromagnetic radiation is consid- ered in this article. The electromagnetic wave penetration mechanism towards the elements of electronic systems and the impact on them are determined by the intensity of the radiation field on the elements of electronic systems. The impact of electromagnetic radiation pulses to the electronic systems refers to physical and analytical parameters of the relationship between exposure to pulses of electromagnetic radiation and the sample parameters of electronic systems. A physical and mathematical model of evaluating the perception level of electronic means to pulsed electromagnetic radiation is given. The developed model was based on the physics of electronics means failure which represents the description of electro- magnetic, electric and thermal processes that lead to the degradation of the original structure of the apparatus elements. The conditions that lead to the total equation electronic systems functional destruction when exposed to electromagnetic radia- tion pulses are described. The internal characteristics of the component elements that respond to the damaging effects are considered. The ratio for the power failure is determined. A thermal breakdown temperature versus pulse duration of expo- sure at various power levels is obtained. The way of evaluation the reliability of electronic systems when exposed to pulses of electromagnetic radiation as a destructive factor is obtained.

  14. A high current, short pulse electron source for wakefield accelerators

    Energy Technology Data Exchange (ETDEWEB)

    Ho, Ching-Hung.

    1992-01-01

    Design studies for the generation of a high current, short pulse electron source for the Argonne Wakefield Accelerator are presented. An L-band laser photocathode rf gun cavity is designed using the computer code URMEL to maximize the electric field on the cathode surface for fixed frequency and rf input power. A new technique using a curved incoming laser wavefront to minimize the space charge effect near the photocathode is studied. A preaccelerator with large iris to minimize wakefield effects is used to boost the drive beam to a useful energy of around 20 MeV for wakefield acceleration experiments. Focusing in the photocathode gun and the preaccelerator is accomplished with solenoids. Beam dynamics simulations throughout the preaccelerator are performed using particle simulation codes TBCI-SF and PARMELA. An example providing a useful set of operation parameters for the Argonne Wakefield Accelerator is given. The effects of the sagitta of the curved beam and laser amplitude and timing jitter effects are discussed. Measurement results of low rf power level bench tests and a high power test for the gun cavity are presented and discussed.

  15. Simulations of pulsed electron beam injection during active experiments

    Science.gov (United States)

    Winglee, R. M.

    1991-01-01

    Two-dimensional electromagnetic particle simulations are used to investigate the characteristics of the spacecraft charging, particle acceleration, and wave emissions during beam injection, turnoff and subsequent pulsing of the beam. It is shown that, during beam injection, the beam current is neutralized by a spatially separate return current region extending several tens of meters from the beam region, with the currents being closed across the field lines by the perpendicular acceleration of ambient plasma ions into the beam region. After beam turnoff, this current system reverses after a time lag of about an ion plasma period. The current reversal is accompanied by prolonged electron collection by the spacecraft near the beam region, preferential ion collection by sections of the spacecraft magnetically connected to the initial return current regions, and the creation of hot plasma extending well into the return current regions. Because of the time lag, the currents induced in the plasma during periodic beam injection can be strongly modified from the imposed beam current.

  16. Pulse-by-pulse multi-beam-line operation for x-ray free-electron lasers

    OpenAIRE

    Toru Hara; Kenji Fukami; Takahiro Inagaki; Hideaki Kawaguchi; Ryota Kinjo; Chikara Kondo; Yuji Otake; Yasuyuki Tajiri; Hideki Takebe; Kazuaki Togawa; Tatsuya Yoshino; Hitoshi Tanaka; Tetsuya Ishikawa

    2016-01-01

    The parallel operation of plural undulator beam lines is an important means of improving the efficiency and usability of x-ray free-electron laser facilities. After the installation of a second undulator beam line (BL2) at SPring-8 Angstrom compact free-electron laser (SACLA), pulse-by-pulse switching between two beam lines was tested using kicker and dc twin-septum magnets. To maintain a compact size, all undulator beam lines at SACLA are designed to be placed within the same undulator hall ...

  17. Instantaneous nonvertical electronic transitions with shaped femtosecond laser pulses: Is it possible?

    DEFF Research Database (Denmark)

    Henriksen, Niels Engholm; Møller, Klaus Braagaard

    2003-01-01

    electronic state. Now, applying pulse shaping via the modulation of the phases of each spectral component of an ultrashort pulse, it is tempting to ask whether it is also possible to induce instantaneous nonvertical transitions to bound electronic states, provided that the phases of each spectral component......In molecular electronic transitions, a vertical transition can be induced by an ultrashort laser pulse. That is, a replica of the initial nuclear state-times the transition dipole moment of the electronic transition-can be created instantaneously (on the time scale of nuclear motion) in the excited...

  18. Nuclear-Motion Effects in Attosecond Transient Absorption Spectroscopy of Molecules

    CERN Document Server

    Bækhøj, Jens E; Madsen, Lars Bojer

    2015-01-01

    We investigate the characteristic effects of nuclear motion on attosecond transient absorption spectra in molecules by calculating the spectrum for different model systems. Two models of the hydrogen molecular ion are considered: one where the internuclear separation is fixed, and one where the nuclei are free to vibrate. The spectra for the fixed nuclei model are similar to atomic spectra reported elsewhere, while the spectra obtained in the model including nuclear motion are very different and dominated by extremely broad absorption features. These broad absorption features are analyzed and their relation to molecular dissociation investigated. The study of the hydrogen molecular ion validates an approach based on the Born-Oppenheimer approximation and a finite electronic basis. This latter approach is then used to study the three-dimensional hydrogen molecule including nuclear vibration. The spectrum obtained from H$_2$ is compared to the result of a fixed-nuclei calculation. In the attosecond transient ab...

  19. Attosecond delay of xenon $4d$ photoionization at the giant resonance and Cooper minimum

    CERN Document Server

    Magrakvelidze, Maia; Chakraborty, Himadri S

    2016-01-01

    A Kohn-Sham time-dependent local-density-functional scheme is utilized to predict attosecond time delays of xenon 4d photoionization that involves the 4d giant dipole resonance and Cooper minimum. The fundamental effect of electron correlations to uniquely determine the delay at both regions is demonstrated. In particular, for the giant dipole resonance, the delay underpins strong collective effect, emulating the recent prediction at C60 giant plasmon resonance [T. Barillot et al, Phys. Rev. A 91, 033413 (2015)]. For the Cooper minimum, a qualitative similarity with a photorecombination experiment near argon 3p minimum [S. B. Schoun et al, Phys. Rev. Lett. 112, 153001 (2014)] is found. The result should encourage attosecond measurements of Xe 4d photoemission.

  20. Direct longitudinal laser acceleration of electrons in free space

    Directory of Open Access Journals (Sweden)

    Sergio Carbajo

    2016-02-01

    Full Text Available Compact laser-driven accelerators are pursued heavily worldwide because they make novel methods and tools invented at national laboratories widely accessible in science, health, security, and technology [V. Malka et al., Principles and applications of compact laser-plasma accelerators, Nat. Phys. 4, 447 (2008]. Current leading laser-based accelerator technologies [S. P. D. Mangles et al., Monoenergetic beams of relativistic electrons from intense laser-plasma interactions, Nature (London 431, 535 (2004; T. Toncian et al., Ultrafast laser-driven microlens to focus and energy-select mega-electron volt protons, Science 312, 410 (2006; S. Tokita et al. Single-shot ultrafast electron diffraction with a laser-accelerated sub-MeV electron pulse, Appl. Phys. Lett. 95, 111911 (2009] rely on a medium to assist the light to particle energy transfer. The medium imposes material limitations or may introduce inhomogeneous fields [J. R. Dwyer et al., Femtosecond electron diffraction: “Making the molecular movie,”, Phil. Trans. R. Soc. A 364, 741 (2006]. The advent of few cycle ultraintense radially polarized lasers [S. Carbajo et al., Efficient generation of ultraintense few-cycle radially polarized laser pulses, Opt. Lett. 39, 2487 (2014] has ushered in a novel accelerator concept [L. J. Wong and F. X. Kärtner, Direct acceleration of an electron in infinite vacuum by a pulsed radially polarized laser beam, Opt. Express 18, 25035 (2010; F. Pierre-Louis et al. Direct-field electron acceleration with ultrafast radially polarized laser beams: Scaling laws and optimization, J. Phys. B 43, 025401 (2010; Y. I. Salamin, Electron acceleration from rest in vacuum by an axicon Gaussian laser beam, Phys. Rev. A 73, 043402 (2006; C. Varin and M. Piché, Relativistic attosecond electron pulses from a free-space laser-acceleration scheme, Phys. Rev. E 74, 045602 (2006; A. Sell and F. X. Kärtner, Attosecond electron bunches accelerated and

  1. A photodiode amplifier system for pulse-by-pulse intensity measurement of an x-ray free electron laser.

    Science.gov (United States)

    Kudo, Togo; Tono, Kensuke; Yabashi, Makina; Togashi, Tadashi; Sato, Takahiro; Inubushi, Yuichi; Omodani, Motohiko; Kirihara, Yoichi; Matsushita, Tomohiro; Kobayashi, Kazuo; Yamaga, Mitsuhiro; Uchiyama, Sadayuki; Hatsui, Takaki

    2012-04-01

    We have developed a single-shot intensity-measurement system using a silicon positive-intrinsic-negative (PIN) photodiode for x-ray pulses from an x-ray free electron laser. A wide dynamic range (10(3)-10(11) photons/pulse) and long distance signal transmission (>100 m) were required for this measurement system. For this purpose, we developed charge-sensitive and shaping amplifiers, which can process charge pulses with a wide dynamic range and variable durations (ns-μs) and charge levels (pC-μC). Output signals from the amplifiers were transmitted to a data acquisition system through a long cable in the form of a differential signal. The x-ray pulse intensities were calculated from the peak values of the signals by a waveform fitting procedure. This system can measure 10(3)-10(9) photons/pulse of ~10 keV x-rays by direct irradiation of a silicon PIN photodiode, and from 10(7)-10(11) photons/pulse by detecting the x-rays scattered by a diamond film using the silicon PIN photodiode. This system gives a relative accuracy of ~10(-3) with a proper gain setting of the amplifiers for each measurement. Using this system, we succeeded in detecting weak light at the developmental phase of the light source, as well as intense light during lasing of the x-ray free electron laser. © 2012 American Institute of Physics

  2. Pulse-periodic generation of supershort avalanche electron beams and X-ray emission

    Science.gov (United States)

    Baksht, E. Kh.; Burachenko, A. G.; Erofeev, M. V.; Tarasenko, V. F.

    2014-05-01

    Pulse-periodic generation of supershort avalanche electron beams (SAEBs) and X-ray emission in nitrogen, as well as the transition from a single-pulse mode to a pulse-periodic mode with a high repetition frequency, was studied experimentally. It is shown that, in the pulse-periodic mode, the full width at halfmaximum of the SAEB is larger and the decrease rate of the gap voltage is lower than those in the single-pulse mode. It is found that, when the front duration of the voltage pulse at a nitrogen pressure of 90 Torr decreases from 2.5 to 0.3 ns, the X-ray exposure dose in the pulse-periodic mode increases by more than one order of magnitude and the number of SAEB electrons also increases. It is shown that, in the pulse-periodic mode of a diffuse discharge, gas heating in the discharge gap results in a severalfold increase in the SAEB amplitude (the number of electrons in the beam). At a generator voltage of 25 kV, nitrogen pressure of 90 Torr, and pulse repetition frequency of 3.5 kHz, a runaway electron beam was detected behind the anode foil.

  3. Generation of femtosecond soft x-ray pulse by interaction between laser and electron beam in an electron storage ring

    CERN Document Server

    Inoue, T; Amano, S; Mochizuki, T; Yatsuzaka, M

    2002-01-01

    A femtosecond synchrotron radiation pulse train can be extracted from an electron storage ring by interaction between an ultrashort laser pulse and an electron beam in an undulator. Generation system of a femtosecond soft x-ray pulse by the slicing technique was studied with numerical calculations for its performance, as applicable for the NewSUBARU synchrotron radiation facility at LASTI. The femtosecond electron pulse, that is energy-modulated with a Ti:sapphire laser at a pulse energy of 100 mu J, a pulse width of 150 fs, and repetition frequency of 20 kHz, can be sufficiently separated in a bending magnet. A femtosecond soft x-ray pulse (the critical photon energy of 0.69 keV and a pulse width of 250 fs) is obtained with a collimator (diameter of 800 mu m phi), and it has an average brightness 3 x 10 sup 6 photons/s/mm sup 2 /mrad sup 2 /0.1 %BW and an average photon flux 10 sup 5 photons/s/0.1 %BW. (author)

  4. Angularly resolved RABBITT using a second harmonic pulse

    Science.gov (United States)

    Loriot, Vincent; Marciniak, Alexandre; Karras, Gabriel; Schindler, Baptiste; Renois-Predelus, Gina; Compagnon, Isabelle; Concina, Bruno; Brédy, Richard; Celep, Gulabi; Bordas, Christian; Constant, Eric; Lépine, Franck

    2017-11-01

    Processes in atoms or molecules on the attosecond timescale have been measured using XUV attosecond and IR femtosecond pulses overlapping in time and controlled with attosecond accuracy. Within this general framework, many strategies have been developed using the harmonics of the fundamental pulse. In this paper, we focus on a specific configuration where the attosecond pulse train is composed by odd harmonics and is dressed by the second harmonic of the fundamental light. Measuring the angularly resolved photoelectron spectrum as a function of the delay between the pulses, a clear oscillation of the anisotropy parameters appears revealing attosecond controlled interferences. This process, is assigned to interferences between two quantum paths involving one XUV photon, on one path, and a XUV+UV photons on the other path. The XUV-UV delay dependent up–down asymmetry can be interpreted following the usual RABBITT formalism, where the dressing photon energy corresponds to the energy separation between the XUV photons of the attosecond pulse train. This approach allows an intuitive analysis of the interference and provides a well suited method for the study of complex valence band systems thanks to the limited congestion of the resulting spectrum.

  5. Pulse energy control through dual loop electronic feedback

    CSIR Research Space (South Africa)

    Jacobs, Cobus

    2006-07-01

    Full Text Available What is Pulse Energy Control: • Reliability & Repeatability • Accuracy & Stability • Programmability head2righthead2rightWhy do we need it: • Protection against component & subject damage • Micromachining with irregular pulse rate • Safer/improved laser....0 20.0 25.0 30.0 35.0 40.0 45.0 50.0 Q-switched Pulse Repetition Rate [Hz] P u l s e E n e r g y [ m J ] Sources of Instability Reliability & Repeatability Programmability Reliability & Repeatability Accuracy & Stability Pump...

  6. Pulse duration and wavelength stability measurements of a midinfrared free-electron laser

    OpenAIRE

    Qin, Yu; Zen, Heishun; Wang, Xiaolong; Kii, Toshiteru; Nakajima, Takashi; Ohgaki, Hideaki

    2013-01-01

    We report the pulse duration and wavelength stability measurements of a midinfrared free-electron laser (FEL) where the wavelength fluctuation may not be negligible. The technique we employ is a fringe-resolved autocorrelation (FRAC) method that has good sensitivity on not only the pulse duration and the chirp but also the wavelength stability. By the simple manipulation of experimental FRAC signals, we can obtain the pulse duration even if the amounts of the chirp and the wavelength stabilit...

  7. Solid-state pulse modulator using Marx generator for a medical linac electron-gun

    Science.gov (United States)

    Lim, Heuijin; Hyeok Jeong, Dong; Lee, Manwoo; Lee, Mujin; Yi, Jungyu; Yang, Kwangmo; Ro, Sung Chae

    2016-04-01

    A medical linac is used for the cancer treatment and consists of an accelerating column, waveguide components, a magnetron, an electron-gun, a pulse modulator, and an irradiation system. The pulse modulator based on hydrogen thyratron-switched pulse-forming network is commonly used in linac. As the improvement of the high power semiconductors in switching speed, voltage rating, and current rating, an insulated gate bipolar transistor has become the more popular device used for pulsed power systems. We propose a solid-state pulse modulator to generator high voltage by multi-stacked storage-switch stages based on the Marx generator. The advantage of our modulator comes from the use of two semiconductors to control charging and discharging of the storage capacitor at each stage and it allows to generate the pulse with various amplitudes, widths, and shapes. In addition, a gate driver for two semiconductors is designed to reduce the control channels and to protect the circuits. It is developed for providing the pulsed power to a medical linac electron-gun that requires 25 kV and 1 A as the first application. In order to improve the power efficiency and achieve the compactness modulator, a capacitor charging power supply, a Marx pulse generator, and an electron-gun heater isolated transformer are constructed and integrated. This technology is also being developed to extend the high power pulsed system with > 1 MW and also other applications such as a plasma immersed ion implantation and a micro pulse electrostatic precipitator which especially require variable pulse shape and high repetition rate > 1 kHz. The paper describes the design features and the construction of this solid-state pulse modulator. Also shown are the performance results into the linac electron-gun.

  8. Pulse-by-pulse multi-beam-line operation for x-ray free-electron lasers

    Directory of Open Access Journals (Sweden)

    Toru Hara

    2016-02-01

    Full Text Available The parallel operation of plural undulator beam lines is an important means of improving the efficiency and usability of x-ray free-electron laser facilities. After the installation of a second undulator beam line (BL2 at SPring-8 Angstrom compact free-electron laser (SACLA, pulse-by-pulse switching between two beam lines was tested using kicker and dc twin-septum magnets. To maintain a compact size, all undulator beam lines at SACLA are designed to be placed within the same undulator hall located downstream of the accelerator. In order to ensure broad tunability of the laser wavelength, the electron bunches are accelerated to different beam energies optimized for the wavelengths of each beam line. In the demonstration, the 30 Hz electron beam was alternately deflected to two beam lines and simultaneous lasing was achieved with 15 Hz at each beam line. Since the electron beam was deflected twice by 3° in a dogleg to BL2, the coherent synchrotron radiation (CSR effects became non-negligible. Currently in a wavelength range of 4–10 keV, a laser pulse energy of 100–150  μJ can be obtained with a reduced peak current of around 1 kA by alleviating the CSR effects. This paper reports the results and operational issues related to the multi-beam-line operation of SACLA.

  9. Electronically driven adsorbate excitation mechanism in femtosecond-pulse laser desorption

    DEFF Research Database (Denmark)

    Brandbyge, Mads; Hedegård, Per; Heinz, T. F.

    1995-01-01

    Femtosecond-pulse laser desorption is a process in which desorption is driven by a subpicosecond temperature pulse of order 5000 K in the substrate-adsorbate electron system, whose energy is transferred into the adsorbate center-of-mass degrees of freedom by a direct coupling mechanism. We presen...

  10. Short energetic electron bunches from laser wakefield accelerator with orthogonally polarized perpendicularly crossed laser pulses

    Science.gov (United States)

    Horný, Vojtěch; Petržílka, Václav; Klimo, Ondřej; Krůs, Miroslav

    2017-05-01

    Electron acceleration with optical injection by a perpendicularly propagating and orthogonally polarized low intensity laser pulse into a nonlinear plasma wave driven by a short intense laser pulse was explored by particle- in-cell simulations. The scheme presented here provides an energetic electron bunch in the first ion cavity with a low energy spread. The electron bunch short and compact, with the mean energy about 400 MeV and a low energy spread about 10 MeV in time of 6 ps of acceleration. The injected charge is several tens of pC for the low intensity of the injection pulse. Initial positions of electrons forming the energetic bunch are shown and then these electrons are followed during the simulation in order to understand the injection process and determine electron bunch properties.

  11. Review of supershort avalanche electron beam during nanosecond-pulse discharges in some gases

    OpenAIRE

    Victor F. Tarasenko; ZHANG Cheng; Baksht, Evgenii Kh.; Burachenko, Alexander G.; Shao, Tao; Dmitry V. Beloplotov; Lomaev, Mikhail I.; Yan, Ping; Kozyrev, Andrey V.; Natalia S. Semeniuk

    2016-01-01

    Supershort avalanche electron beam (SAEB) plays an important role in nanosecond-pulse discharges. This paper aims at reviewing experiments results on characteritics of SAEB and its spectra in different gases in nanosecond-pulse discharges. All the joint experiments were carried in the Institute of High Current Electronics of the Russian Academy of Sciences and the Institute of Electrical Engineering of the Chinese Academy of Sciences. In these experiments, the generation of a SAEB in SF6 in a...

  12. Time delays for attosecond streaking in photoionization of neon

    CERN Document Server

    Feist, Johannes; Nagele, Stefan; Pazourek, Renate; Burgdörfer, Joachim; Guan, Xiaoxu; Bartschat, Klaus; Schneider, Barry I

    2014-01-01

    We revisit the time-resolved photoemission in neon atoms as probed by attosecond streaking. We calculate streaking time shifts for the emission of 2p and 2s electrons and compare the relative delay as measured in a recent experiment by Schultze et al. [Science 328, 1658 (2010)]. The B-spline R-matrix method is employed to calculate accurate Eisenbud-Wigner-Smith time delays from multi- electron dipole transition matrix elements for photoionization. The additional laser field-induced time shifts in the exit channel are obtained from separate, time-dependent simulations of a full streaking process by solving the time-dependent Schr\\"odinger equation on the single-active-electron level. The resulting accurate total relative streaking time shifts between 2s and 2p emission lie well below the experimental data. We identify the presence of unresolved shake-up satellites in the experiment as a potential source of error in the determination of streaking time shifts.

  13. On the response of electronic personal dosimeters in constant potential and pulsed X-ray beams

    Energy Technology Data Exchange (ETDEWEB)

    Guimaraes, Margarete C.; Silva, Teogenes; Silva, Claudete R.E., E-mail: margaretecristinag@gmail.com [Centro de Desenvolvimento da Tecnologia Nuclear (CDTN/CNEN-MG), Belo Horizonte, MG (Brazil); Oliveira, Paulo Marcio C. de [Universidade Federal de Minas Gerais (UFMG), Belo Horizonte, MG (Brazil). Departamento de Anatomia e Imagem

    2015-07-01

    Electronic personal dosimeters (EPDs) based on solid state detectors have widely been used but some deficiencies in their response in pulsed radiation beams have been reported. Nowadays, there is not an international standard for pulsed X-ray beams for calibration or type testing of dosimeters. Irradiation conditions for testing the response of EPDs in both the constant potential and pulsed X-ray beams were established in CDTN. Three different types of EPDs were tested in different conditions in similar ISO and IEC X-ray qualities. Results stressed the need of performing additional checks before using EPDs in constant potential or pulsed X-rays. (author)

  14. Intense ultrashort pulse generation using the JAERI far-infrared free electron laser

    CERN Document Server

    Nagai, R; Nishimori, N; Kikuzawa, N; Sawamura, M; Minehara, E J

    2002-01-01

    An intense ultrashort optical pulse has been quasi-continuously generated using a superconducting RF linac-based free-electron laser at a wavelength of 22.5 mu m. The pulse shape and width are measured by second-order optical autocorrelation with a birefringent Te crystal. At synchronism of the optical resonator, the pulse shape is a smooth single pulse with an FWHM width of 255 fs and energy of 74 mu J. A train of subpulses is developed by increasing the desynchronism of the optical resonator. The measured results are in good agreement with numerical simulation.

  15. Plasmonic pulse shaping and velocity control via photoexcitation of electrons in a gold film.

    Science.gov (United States)

    Khokhlov, Nikola E; Ignatyeva, Daria O; Belotelov, Vladimir I

    2014-11-17

    We study the possibility of surface plasmon polariton (SPP) pulse shape, delay and duration manipulation on sub-picosecond timescales via a high intensity pump SPP pulse photoexciting electrons in a gold film. We present a theoretical model describing this process and show that the pump induces the phase modulation of the probe pulse leading to its compression by about 20% and the variation of the delay between two SPP pulses up to 15 fs for the incident fluence of the pump of 1.5 mJ∙cm⁻².

  16. Effect of pulse-modulated microwaves on fullerene ion production with electron cyclotron resonance ion source.

    Science.gov (United States)

    Asaji, T; Uchida, T; Minezaki, H; Oshima, K; Racz, R; Muramatsu, M; Biri, S; Kitagawa, A; Kato, Y; Yoshida, Y

    2012-02-01

    Fullerene plasmas generated by pulse-modulated microwaves have been investigated under typical conditions at the Bio-Nano electron cyclotron resonance ion source. The effect of the pulse modulation is distinct from that of simply structured gases, and then the density of the fullerene plasmas increased as decreasing the duty ratio. The density for a pulse width of 10 μs at the period of 100 μs is 1.34 times higher than that for CW mode. We have studied the responses of fullerene and argon plasmas to pulsed microwaves. After the turnoff of microwave power, fullerene plasmas lasted ∼30 times longer than argon plasmas.

  17. Attosecond spectroscopy of autoionizing states

    OpenAIRE

    Jiménez Galán, Álvaro

    2015-01-01

    Tesis doctoral inédita leída en la Universidad Autónoma de Madrid, Facultad de Ciencias, Departamento de Química. Fecha de lectura: 15-12-2015 In this PhD Thesis we report a theoretical time-resolved study of the effects of electron correlation in the single photoionization spectrum of atomic systems, with particular focus on multi-photon transitions occurring in the presence of autoionizing states. For this task, we take two complementary approaches. On the one hand, we solve ...

  18. Electron yield enhancement in a laser wakefield accelerator driven by asymmetric laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Leemans, W.P.; Catravas, P.; Esarey, E.; Geddes, C.G.R.; Toth, C.; Trines, R.; Schroeder, C.B.; Shadwick, B.A.; van Tilborg, J.; Faure, J.

    2002-08-01

    The effect of asymmetric laser pulses on electron yield from a laser wakefield accelerator has been experimentally studied using > 10{sup 19} cm{sup -3} plasmas and a 10 TW, > 45 fs, Ti:Al{sub 2}O{sub 3} laser. Laser pulse shape was controlled through non-linear chirp with a grating pair compressor. Pulses (76 fs FWHM) with a steep rise and positive chirp were found to significantly enhance the electron yield compared to pulses with a gentle rise and negative chirp. Theory and simulation show that fast rising pulses can generate larger amplitude wakes that seed the growth of the self-modulation instability and that frequency chirp is of minimal importance for the experimental parameters.

  19. Vacuum ultraviolet circularly polarized coherent femtosecond pulses from laser seeded relativistic electrons

    Directory of Open Access Journals (Sweden)

    N. Čutić

    2011-03-01

    Full Text Available We have demonstrated the generation of circularly polarized coherent light pulses at 66 nm wavelength by combining laser seeding at 263 nm of a 375 MeV relativistic electron bunch with subsequent coherent harmonic generation from an elliptical undulator of APPLE-II type. Coherent pulses at higher harmonics in linear polarization have been produced and recorded up to the sixth order (44 nm. The duration of the generated pulses depends on the temporal overlap of the initial seed laser pulse and the electron bunch and was on the order of 200 fs. Currently, this setup is the only source worldwide producing coherent fs-light pulses with variable polarization in the vacuum ultraviolet.

  20. Charge collection efficiency in ionization chambers exposed to electron beams with high dose per pulse.

    Science.gov (United States)

    Laitano, R F; Guerra, A S; Pimpinella, M; Caporali, C; Petrucci, A

    2006-12-21

    The correction for charge recombination was determined for different plane-parallel ionization chambers exposed to clinical electron beams with low and high dose per pulse, respectively. The electron energy was nearly the same (about 7 and 9 MeV) for any of the beams used. Boag's two-voltage analysis (TVA) was used to determine the correction for ion losses, k(s), relevant to each chamber considered. The presence of free electrons in the air of the chamber cavity was accounted for in determining k(s) by TVA. The determination of k(s) was made on the basis of the models for ion recombination proposed in past years by Boag, Hochhäuser and Balk to account for the presence of free electrons. The absorbed dose measurements in both low-dose-per-pulse (less than 0.3 mGy per pulse) and high-dose-per-pulse (20-120 mGy per pulse range) electron beams were compared with ferrous sulphate chemical dosimetry, a method independent of the dose per pulse. The results of the comparison support the conclusion that one of the models is more adequate to correct for ion recombination, even in high-dose-per-pulse conditions, provided that the fraction of free electrons is properly assessed. In this respect the drift velocity and the time constant for attachment of electrons in the air of the chamber cavity are rather critical parameters because of their dependence on chamber dimensions and operational conditions. Finally, a determination of the factor k(s) was also made by zero extrapolation of the 1/Q versus 1/V saturation curves, leading to the conclusion that this method does not provide consistent results in high-dose-per-pulse beams.

  1. Free-electron-laser-induced shock-wave control and mechanistic analysis using pulse control.

    Science.gov (United States)

    Kanai, Taizo; Yoshihashi-Suzuki, Sachiko; Awazu, Kunio

    2008-11-01

    The wavelength of the free electron laser (FEL) in Osaka University can be continuously varied in the range of 5.0-20.0 microm. The FEL has a double-pulse structure, consisting of a train of macropulses of pulse duration 12 micros. Each macropulse contains a train of 330 micropulses of pulse duration 5 ps. The tunability and picosecond pulses afford new medical and biological applications. However, a macropulse of long pulse duration leads to undesirable secondary effects. Precise control of the macropulse duration is essential for the high-precision applications of the FEL. An FEL pulse control system using acousto-optic modulators has been developed to investigate mechanical (shock-wave) effects of the FEL on living tissues. With this system, we have controlled photoinduced shock waves and determine the mechanism of interaction during FEL-induced tissue ablation.

  2. Electron injection and emittance control by transverse colliding pulses in a laser-plasma accelerator

    Directory of Open Access Journals (Sweden)

    M. Chen

    2014-05-01

    Full Text Available A method to inject electron beams with controllable transverse emittances in a laser-plasma accelerators is proposed and analyzed. It uses two colliding laser pulses that propagate transversely to the plasma wave. For colliding pulses with equal frequencies, a beam with very low emittance is generated when the collision is close to the density peak of the plasma wave. Electrons near the axis are accelerated longitudinally by the ponderomotive force of the colliding pulses, accelerated transversely by the beat wave, and subsequently injected into the second bucket of the wake. Ionization is used to increase the transverse injection area and the final trapped charge. Simulations show that the transverse emittance can be less than the 0.1 mm mrad level, which is important for many applications. For colliding laser pulses with different frequencies, the beat wave can produce asymmetric injection, which can enhance betatron radiation generated by the electron beam.

  3. Attosecond polarization control in atomic RABBITT-like experiments assisted by a circularly polarized laser

    Science.gov (United States)

    Boll, D. I. R.; Fojón, O. A.

    2017-12-01

    We study theoretically the single ionization of noble gas atoms by the combined action of an attosecond pulse train with linear polarization and an assistant laser field with circular polarization. We employ a non-perturbative model that under certain approximations gives closed-form expressions for the angular distributions of photoelectrons. Interestingly, our model allow us to interpret these angular distributions as two-centre interferences where the orientation and the modulus of the separation vector between the virtual emitters is governed by the assistant laser field. Additionally, we show that such a configuration of light fields is similar to the polarization control technique, where both the attosecond pulse train and the assistant laser field have linear polarizations whose relative orientation may be controlled. Moreover, in order to compare our results with the available experimental data, we obtain analytical expressions for the cross sections integrated over the photoelectron emission angles. By means of these expressions, we define the ‘magic time’ as the delay for which the total cross sections for atomic targets exhibit the same functional form as the one of the monochromatic photoionization of diatomic molecular targets.

  4. Relativistic Electron Acceleration with Ultrashort Mid-IR Laser Pulses

    Science.gov (United States)

    Feder, Linus; Woodbury, Daniel; Shumakova, Valentina; Gollner, Claudia; Miao, Bo; Schwartz, Robert; Pugžlys, Audrius; Baltuška, Andrius; Milchberg, Howard

    2017-10-01

    We report the first results of laser plasma wakefield acceleration driven by ultrashort mid-infrared laser pulses (λ = 3.9 μm , pulsewidth 100 fs, energy width, as well as trends in the accelerated beam profiles, charge and energy spectra which are supported by 3D particle-in-cell simulations. These results extend earlier work with sub-TW self-modulated laser wakefield acceleration using near IR drivers to the Mid-IR, and enable us to capture time-resolved images of relativistic self-focusing of the laser pulse. This work supported by DOE (DESC0010706TDD, DESC0015516); AFOSR(FA95501310044, FA95501610121); NSF(PHY1535519); DHS.

  5. Quantum computers based on electron spins controlled by ultrafast off-resonant single optical pulses.

    Science.gov (United States)

    Clark, Susan M; Fu, Kai-Mei C; Ladd, Thaddeus D; Yamamoto, Yoshihisa

    2007-07-27

    We describe a fast quantum computer based on optically controlled electron spins in charged quantum dots that are coupled to microcavities. This scheme uses broadband optical pulses to rotate electron spins and provide the clock signal to the system. Nonlocal two-qubit gates are performed by phase shifts induced by electron spins on laser pulses propagating along a shared waveguide. Numerical simulations of this scheme demonstrate high-fidelity single-qubit and two-qubit gates with operation times comparable to the inverse Zeeman frequency.

  6. Experiments on Ion Beam Space-Charge Neutralization with Pulsed Electron Beams

    CERN Document Server

    Herleb, U

    1998-01-01

    Space-charge neutralization of heavy ion beams with electron beam pulses generated by electron guns incorporating ferroelectric cathodes has been experimentally investigated. Several experiments are described, the results of which prove that the intensity of selected ion beam parts with defined charge states generated in a laser ion source can be increased by an order of magnitude. For elevated charge states the intensity amplification is more significant than for low charge states. A charge enhancement factor of four has been achieved by neutralization with pulsed electron beams for Al7+ ions generated from an aluminium target.

  7. Pulse length of ultracold electron bunches extracted from a laser cooled gas

    Science.gov (United States)

    Franssen, J. G. H.; Frankort, T. L. I.; Vredenbregt, E. J. D.; Luiten, O. J.

    2017-01-01

    We present measurements of the pulse length of ultracold electron bunches generated by near-threshold two-photon photoionization of a laser-cooled gas. The pulse length has been measured using a resonant 3 GHz deflecting cavity in TM110 mode. We have measured the pulse length in three ionization regimes. The first is direct two-photon photoionization using only a 480 nm femtosecond laser pulse, which results in short (∼15 ps) but hot (∼104 K) electron bunches. The second regime is just-above-threshold femtosecond photoionization employing the combination of a continuous-wave 780 nm excitation laser and a tunable 480 nm femtosecond ionization laser which results in both ultracold (∼10 K) and ultrafast (∼25 ps) electron bunches. These pulses typically contain ∼103 electrons and have a root-mean-square normalized transverse beam emittance of 1.5 ± 0.1 nm rad. The measured pulse lengths are limited by the energy spread associated with the longitudinal size of the ionization volume, as expected. The third regime is just-below-threshold ionization which produces Rydberg states which slowly ionize on microsecond time scales. PMID:28396879

  8. The Boersch effect in a picosecond pulsed electron beam emitted from a semiconductor photocathode

    Energy Technology Data Exchange (ETDEWEB)

    Kuwahara, Makoto, E-mail: kuwahara@imass.nagoya-u.ac.jp; Ujihara, Toru; Saitoh, Koh [Institute of Materials and Systems for Sustainability, Nagoya University, Nagoya 464-8603 (Japan); Graduate School of Engineering, Nagoya University, Nagoya 464-8603 (Japan); Nambo, Yoshito; Aoki, Kota; Sameshima, Kensuke; Asano, Hidefumi [Graduate School of Engineering, Nagoya University, Nagoya 464-8603 (Japan); Jin, Xiuguang [High Energy Accelerator Research Organization (KEK), Tsukuba 305-0801 (Japan); Takeda, Yoshikazu [Aichi Synchrotron Radiation Center, Seto 489-0965 (Japan); Nagoya Industrial Science Research Institute, Nagoya 460-0008 (Japan); Tanaka, Nobuo [Institute of Materials and Systems for Sustainability, Nagoya University, Nagoya 464-8603 (Japan)

    2016-07-04

    The space charge effect has been clearly observed in the energy distributions of picosecond pulse beams from a spin-polarized electron microscope, and was found to depend upon the quantity of charge per pulse. The non-linear phenomena associated with this effect have also been replicated in beam simulations that take into account of a three-dimensional space charge. The results show that a charge of 500 aC/pulse provides the highest brightness with a 16-ps pulse duration, a 30-keV beam energy, and an emission spot of 1.8 μm. Furthermore, the degeneracy of the wave packet of the pulsed electron beam has been evaluated to be 1.6 × 10{sup −5} with a charge of 100 aC/pulse, which is higher than that for a continuously emitted electron beam despite the low beam energy of 30 keV. The high degeneracy and high brightness contribute to the realization of high temporal and energy resolutions in low-voltage electron microscopy, which will serve to reduce radiolysis damage and enhance scattering contrast.

  9. Ultrashort laser pulse-induced anti-Stokes photoluminescence of hot electrons in gold nanorods

    Science.gov (United States)

    Sitnikov, D. S.; Yurkevich, A. A.; Kotelev, M. S.; Ziangirova, M.; Chefonov, O. V.; Ilina, I. V.; Vinokurov, V. A.; Muradov, A. V.; Itzkan, I.; Agranat, M. B.; Perelman, L. T.

    2014-07-01

    We report observing anti-Stokes broadband radiation induced in gold nanorods by ultrashort laser pulses. The radiation is in the visible spectral range along with the second harmonic peak. Unlike conventional photoluminescence of metal nanoparticles, the energy of the excitation photons is smaller than the gap between the top of the d band and the Fermi level. Because the gold nanorods are irradiated with a pulse whose time is shorter than the electron-phonon equilibration time in gold, the energy is absorbed by s/p band electrons, creating a temperature difference between the electrons and the lattice, as described by the two-temperature model. Therefore, we identify the origin of the observed radiation as the recombination of hot conduction electrons with the d band holes created by the same ultrashort laser pulse.

  10. Ecton processes in the generation of pulsed runaway electron beams in a gas discharge

    Science.gov (United States)

    Mesyats, G. A.

    2017-09-01

    As was shown earlier for pulsed discharges that occur in electric fields rising with extremely high rates (1018 V/(cm s)) during the pulse rise time, the electron current in a vacuum discharge is lower than the current of runaway electrons in an atmospheric air discharge in a 1-cm-long gap. In this paper, this is explained by that the field emission current from cathode microprotrusions in a gas discharge is enhanced due to gas ionization. This hastens the initiation of explosive electron emission, which occurs within 10-11 s at a current density of up to 1010 A/cm2. Thereafter, a first-type cathode spot starts forming. The temperature of the cathode spot decreases due to heat conduction, and the explosive emission current ceases. Thus, the runaway electron current pulse is similar in nature to the ecton phenomenon in a vacuum discharge.

  11. Flexible attosecond beamline for high harmonic spectroscopy and XUV/near-IR pump probe experiments requiring long acquisition times

    Science.gov (United States)

    Weber, S. J.; Manschwetus, B.; Billon, M.; Böttcher, M.; Bougeard, M.; Breger, P.; Géléoc, M.; Gruson, V.; Huetz, A.; Lin, N.; Picard, Y. J.; Ruchon, T.; Salières, P.; Carré, B.

    2015-03-01

    We describe the versatile features of the attosecond beamline recently installed at CEA-Saclay on the PLFA kHz laser. It combines a fine and very complete set of diagnostics enabling high harmonic spectroscopy (HHS) through the advanced characterization of the amplitude, phase, and polarization of the harmonic emission. It also allows a variety of photo-ionization experiments using magnetic bottle and COLTRIMS (COLd Target Recoil Ion Momentum Microscopy) electron spectrometers that may be used simultaneously, thanks to a two-foci configuration. Using both passive and active stabilization, special care was paid to the long term stability of the system to allow, using both experimental approaches, time resolved studies with attosecond precision, typically over several hours of acquisition times. As an illustration, applications to multi-orbital HHS and electron-ion coincidence time resolved spectroscopy are presented.

  12. Surface cracking of soda lime glass under pulsed high-current electron radiation

    Energy Technology Data Exchange (ETDEWEB)

    Wang, Paul W. [Department of Physics, Bradley University, Peoria, IL 61625 (United States)]. E-mail: pwang@bradley.edu; Kimberlin, K.R. [Department of Physics, Bradley University, Peoria, IL 61625 (United States); Wang Chengyu [Institute of Glass and Inorganic New Materials, Dalian Institute of Light Industry (China); Tao Ying [Institute of Glass and Inorganic New Materials, Dalian Institute of Light Industry (China); Guo Quianglin [Laboratory of Material Modification by Ion, Electron, and Laser Beam, Dalian University of Technology (China); Wu Aimin [Laboratory of Material Modification by Ion, Electron, and Laser Beam, Dalian University of Technology (China); Xu Jiujun [Institute of Materials and Technology, Dalian Maritime University (China)

    2005-12-15

    Electron beam radiation has been widely used to modify the surface properties of materials such as metals, ceramics, and glasses. However, a few investigations of surface topology of glasses after electron irradiation can be found. In contrast to the surface cracking by bending, indentation, and thermally induced stress in soda lime glasses a 2 {mu}s pulsed high-current electron beam was used to modify the surfaces of soda lime glass. Surface topology of irradiated samples was studied by using traditional optical microscopy and atomic force microscopy. Parallel to and perpendicular to surface cracks were observed. The depth of crack can be obtained by electron penetration, Newton's ring and AFM. The stress to produce the crack by electron radiation was calculated using three obtained depths. The observed surface crack is explained in terms of radiation-induced thermal stress and high local electric field-induced by deposited charges from pulsed electrons.

  13. Multichannel computerized control system of current pulses in LIU-30 electron accelerator

    CERN Document Server

    Gerasimov, A I; Kulgavchuk, V V; Pluzhnikov, A V

    2002-01-01

    In LIU-30 power linear pulsed induction electron accelerator (40 MeV, 10 kA, 25 ns) 288 radial lines with water insulation serve as energy accumulators and shapers of accelerating voltage pulses. The lines are charged simultaneously up to 500 kV using a system comprising 72 Arkadiev-Marx screened generators. To control parameter of synchronous pulses of charging current with up to 60 kA amplitude and 0.85 mu s duration in every of 72 charging circuits one applies a computer-aided system. Current pulse is recorded at output of every generator using the Rogowski coil signal from which via a cable line is transmitted to an analog-digital converter, is processed with 50 ns sampling and is recorded to a memory unit. Upon actuation of accelerator the signals are sequentially or selectively displayed and are compared with pulse typical shape

  14. Spectrum of fast electrons in a dense gas in the presence of a nonuniform pulsed field

    Science.gov (United States)

    Tkachev, A. N.; Yakovlenko, S. I.

    2007-01-01

    The problems of gas preionization in discharges related to laser physics are considered. The propagation of fast electrons injected from the cathode in the presence of a nonuniform nonstationary field and the motion of multiplying electrons at the edge of the avalanche in the presence of a nonuniform nonstationary field are simulated. The effect of the voltage pulse steepness and the field nonuniformity on the mean propagation velocity of fast electrons and their energy distribution is demonstrated. At certain combinations of the voltage pulse rise time and amplitude and at a certain time interval, the center of gravity of the electron cloud can move in the opposite direction relative to the direction of force acting upon electrons. It is also demonstrated that the number of hard particles (and, hence, the hard component of the x-ray bremsstrahlung) increases with both an increase in the voltage amplitude and a decrease in the pulse rise time. For nonoptimal conditions of the picosecond voltage pulse, an assumption is formulated: an electron beam in gas is formed due to the electrons at the edge of the avalanche rather than the background multiplication wave approaching the anode.

  15. Paired-pulse facilitation achieved in protonic/electronic hybrid indium gallium zinc oxide synaptic transistors

    OpenAIRE

    Li Qiang Guo; Li Qiang Zhu; Jian Ning Ding; Yu Kai Huang

    2015-01-01

    Neuromorphic devices with paired pulse facilitation emulating that of biological synapses are the key to develop artificial neural networks. Here, phosphorus-doped nanogranular SiO2 electrolyte is used as gate dielectric for protonic/electronic hybrid indium gallium zinc oxide (IGZO) synaptic transistor. In such synaptic transistors, protons within the SiO2 electrolyte are deemed as neurotransmitters of biological synapses. Paired-pulse facilitation (PPF) behaviors for the analogous informati...

  16. Production and application of pulsed slow-positron beam using an electron LINAC

    Energy Technology Data Exchange (ETDEWEB)

    Yamazaki, Tetsuo; Suzuki, Ryoichi; Ohdaira, Toshiyuki; Mikado, Tomohisa [Electrotechnical Lab., Tsukuba, Ibaraki (Japan); Kobayashi, Yoshinori

    1997-03-01

    Slow-positron beam is quite useful for non-destructive material research. At the Electrotechnical Laboratory (ETL), an intense slow positron beam line by exploiting an electron linac has been constructed in order to carry out various experiments on material analysis. The beam line can generates pulsed positron beams of variable energy and of variable pulse period. Many experiments have been carried out so far with the beam line. In this paper, various capability of the intense pulsed positron beam is presented, based on the experience at the ETL, and the prospect for the future is discussed. (author)

  17. Solid-state pulsed microwave bridge for electron spin echo spectrometers of 8-mm wavelength range

    Directory of Open Access Journals (Sweden)

    Kalabukhova E. N.

    2012-12-01

    Full Text Available The article presents a construction of a coherent pulsed microwave bridge with an output power up to 10 Wt with a time resolution of 10–8 seconds at a pulse repetition rate of 1 kHz designed for electron spin echo spectrometers. The bridge is built on a homodyne scheme based on IMPATT diodes, which are used for modulation and amplification of microwave power coming from the reference Gunn diode oscillator. The advantages of the bridge are optimal power and minimum pulse width, simple operation, low cost.

  18. Pulsed cathodoluminescence of diamond, calcite, spodumene, and fluorite under the action of subnanosecond electron beam

    Science.gov (United States)

    Baksht, E. Kh.; Burachenko, A. G.; Tarasenko, V. F.

    2010-11-01

    Amplitude and temporal characteristics of pulsed cathodoluminescence (PCL) of diamond (natural and synthetic), calcite, spodumene, and fluorite have been studied at a temporal resolution of ˜0.3 ns. The PCL was generated by electron beam pulses with a full width at half maximum (FWHM) of 0.1, 0.25, and 0.65 ns. The PCL spectra have been measured for the emission induced by 0.1- and 0.25-ns pulses at a beam current density of ˜90 A/cm2.

  19. Beat wave injection of electrons into plasma waves using two interfering laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Fubiani, G.; Esarey, E.; Schroeder, C.B.; Leemans, W.P.

    2004-03-04

    An electron injector concept that uses a single injection laser pulse colliding with a pump laser pulse in a plasma is analyzed. The pump pulse generates a large amplitude laser wakefield (plasma wave). The counter propagating injection pulse collides with the pump laser pulse to generate a beat wave with a slow phase velocity. The ponderomotive force of the slow beat wave is responsible for injecting plasma electrons into the wakefield near the back of the pump pulse. Test particle simulations indicate that significant amounts of charge can be trapped and accelerated ({approx} 10 pC). For higher charge, beam loading limits the validity of the simulations. The accelerated bunches are ultrashort ({approx} 1 fs) with good beam quality (relative energy spread of a few percent at a mean energy of {approx} 10 MeV and a normalized rms emittance on the order 0.4 mm.mrad). The effects of interaction angle and polarization are also explored, e.g., efficient trapping can occur for near-collinear geometries. Beat wave injection using a single injection pulse has the advantages of simplicity, ease of experimental implementation, and requires modest laser intensity I {approx_equal} 8.8 x 10{sup 17} W/cm{sup 2}.

  20. Generation of stable subfemtosecond hard x-ray pulses with optimized nonlinear bunch compression

    Directory of Open Access Journals (Sweden)

    Senlin Huang

    2014-12-01

    Full Text Available In this paper, we propose a simple scheme that leverages existing x-ray free-electron laser hardware to produce stable single-spike, subfemtosecond x-ray pulses. By optimizing a high-harmonic radio-frequency linearizer to achieve nonlinear compression of a low-charge (20 pC electron beam, we obtain a sharp current profile possessing a few-femtosecond full width at half maximum temporal duration. A reverse undulator taper is applied to enable lasing only within the current spike, where longitudinal space charge forces induce an electron beam time-energy chirp. Simulations based on the Linac Coherent Light Source parameters show that stable single-spike x-ray pulses with a duration less than 200 attoseconds can be obtained.

  1. Electron energy distributions and electron impact source functions in Ar/N{sub 2} inductively coupled plasmas using pulsed power

    Energy Technology Data Exchange (ETDEWEB)

    Logue, Michael D., E-mail: mdlogue@umich.edu; Kushner, Mark J., E-mail: mjkush@umich.edu [Department of Electrical Engineering and Computer Science, University of Michigan, 1301 Beal Ave., Ann Arbor, Michigan 48109-2122 (United States)

    2015-01-28

    In plasma materials processing, such as plasma etching, control of the time-averaged electron energy distributions (EEDs) in the plasma allows for control of the time-averaged electron impact source functions of reactive species in the plasma and their fluxes to surfaces. One potential method for refining the control of EEDs is through the use of pulsed power. Inductively coupled plasmas (ICPs) are attractive for using pulsed power in this manner because the EEDs are dominantly controlled by the ICP power as opposed to the bias power applied to the substrate. In this paper, we discuss results from a computational investigation of EEDs and electron impact source functions in low pressure (5–50 mTorr) ICPs sustained in Ar/N{sub 2} for various duty cycles. We find there is an ability to control EEDs, and thus source functions, by pulsing the ICP power, with the greatest variability of the EEDs located within the skin depth of the electromagnetic field. The transit time of hot electrons produced in the skin depth at the onset of pulse power produces a delay in the response of the EEDs as a function of distance from the coils. The choice of ICP pressure has a large impact on the dynamics of the EEDs, whereas duty cycle has a small influence on time-averaged EEDs and source functions.

  2. Experimental Study of RF Pulsed Heating on Oxygen Free Electronic Copper

    Energy Technology Data Exchange (ETDEWEB)

    Pritzkau, David P.

    2003-02-10

    When the thermal stresses induced by RF pulsed heating are larger than the elastic limit, microcracks and surface roughening will occur due to cyclic fatigue. Therefore, pulsed heating limits the maximum surface magnetic field and through it the maximum achievable accelerating gradient. An experiment using circularly cylindrical cavities operating in the TE{sub 011} mode at a resonant frequency of 11.424 GHz was designed to study pulsed heating on Oxygen Free Electronic (OFE) copper. An X-band klystron delivered up to 10 MW to the cavities in 1.5 {micro}s pulses at 60 Hz repetition rate. One run was executed at a temperature rise of 120 K for 56 x 10{sup 6} pulses. Cracks at grain boundaries, slip bands and cracks associated with these slip bands were observed. The second run consisted of 86 x 10{sup 6} pulses with a temperature rise of 82 K, and cracks at grain boundaries and slip bands were seen. Additional information can be derived from the power-coupling iris, and we conclude that a pulsed temperature rise of 250 K for several million pulses leads to destruction of copper. These results can be applied to any mode of any OFE copper cavity.

  3. Generation of large-bandwidth x-ray free-electron-laser pulses

    Directory of Open Access Journals (Sweden)

    Angela Saa Hernandez

    2016-09-01

    Full Text Available X-ray free-electron lasers (XFELs are modern research tools in disciplines such as biology, material science, chemistry, and physics. Besides the standard operation that aims at minimizing the bandwidth of the produced XFEL radiation, there is a strong scientific demand to produce large-bandwidth XFEL pulses for several applications such as nanocrystallography, stimulated Raman spectroscopy, and multiwavelength anomalous diffraction. We present a self-consistent method that maximizes the XFEL pulse bandwidth by systematically maximizing the energy chirp of the electron beam at the undulator entrance. This is achieved by optimizing the compression scheme and the electron distribution at the source in an iterative back-and-forward tracking. Start-to-end numerical simulations show that a relative bandwidth of 3.25% full-width can be achieved for the hard x-ray pulses in the SwissFEL case.

  4. Effect of pulsed hollow electron-lens operation on the proton beam core in LHC

    Energy Technology Data Exchange (ETDEWEB)

    Fitterer, Miriam [Fermi National Accelerator Lab. (FNAL), Batavia, IL (United States); Stancari, Giulio [Fermi National Accelerator Lab. (FNAL), Batavia, IL (United States); Valishev, Alexander [Fermi National Accelerator Lab. (FNAL), Batavia, IL (United States)

    2016-11-08

    Collimation with hollow electron beams is currently one of the most promising concepts for active halo control in the HL-LHC. In order to further increase the diffusion rates for a fast halo removal as e.g. desired before the squeeze, the electron lens (e-lens) can be operated in pulsed mode. In case of profile imperfections in the electron beam the pulsing of the e-lens induces noise on the proton beam which can, depending on the frequency content and strength, lead to emittance growth. In order to study the sensitivity to the pulsing pattern and the amplitude, a beam study (machine development MD) at the LHC has been proposed for August 2016 and we present in this note the preparatory simulations and estimates.

  5. Effect of pulsed hollow electron-lens operation on the proton beam core in LHC

    CERN Document Server

    Fitterer, Miriam; Valishev, Alexander

    2016-01-01

    Collimation with hollow electron beams is currently one of the most promising concepts for active halo control in the HL-LHC. In order to further increase the diffusion rates for a fast halo removal as e.g. desired before the squeeze, the electron lens (e-lens) can be operated in pulsed mode. In case of profile imperfections in the electron beam the pulsing of the e-lens induces noise on the proton beam which can, depending on the frequency content and strength, lead to emittance growth. In order to study the sensitivity to the pulsing pattern and the amplitude, a beam study (machine development MD) at the LHC has been proposed for August 2016 and we present in this note the preparatory simulations and estimates.

  6. Hot electron production in laser solid interactions with a controlled pre-pulse

    Energy Technology Data Exchange (ETDEWEB)

    Culfa, O.; Tallents, G. J.; Wagenaars, E.; Ridgers, C. P.; Dance, R. J.; Rossall, A. K.; Woolsey, N. C. [York Plasma Institute, Department of Physics, The University of York, York YO10 5DD (United Kingdom); Gray, R. J.; McKenna, P. [Department of Physics, SUPA, University of Strathclyde, Glasgow G4 0NG (United Kingdom); Brown, C. D. R.; James, S. F.; Hoarty, D. J. [AWE, Aldermaston, Reading, Berkshire RG7 4PR (United Kingdom); Booth, N.; Robinson, A. P. L. [CLF, STFC Rutherford Appleton Laboratory, Didcot, Oxfordshire OX11 0QX (United Kingdom); Lancaster, K. L. [York Plasma Institute, Department of Physics, The University of York, York YO10 5DD (United Kingdom); CLF, STFC Rutherford Appleton Laboratory, Didcot, Oxfordshire OX11 0QX (United Kingdom); Pikuz, S. A. [Joint Institute for High Temperatures, Russian Academy of Sciences, Moscow 125412 (Russian Federation); Faenov, A. Ya. [Joint Institute for High Temperatures, Russian Academy of Sciences, Moscow 125412 (Russian Federation); Quantum Beam Science Directorate, Japan Atomic Energy Agency, Kizugawa, Kyoto 619-0215 (Japan); Kampfer, T.; Schulze, K. S.; Uschmann, I. [Friedrich Schiller University of Jena, D-07743 Jena (Germany)

    2014-04-15

    Hot electron generation plays an important role in the fast ignition approach to inertial confinement fusion (ICF) and other applications with ultra-intense lasers. Hot electrons of temperature up to 10–20 MeV have been produced by high contrast picosecond duration laser pulses focussed to intensities of ∼10{sup 20} W cm{sup −2} with a deliberate pre-pulse on solid targets using the Vulcan Petawatt Laser facility. We present measurements of the number and temperature of hot electrons obtained using an electron spectrometer. The results are correlated to the density scale length of the plasma produced by a controlled pre-pulse measured using an optical probe diagnostic. 1D simulations predict electron temperature variations with plasma density scale length in agreement with the experiment at shorter plasma scale lengths (<7.5μm), but with the experimental temperatures (13–17 MeV) dropping below the simulation values (20–25 MeV) at longer scale lengths. The experimental results show that longer interaction plasmas produced by pre-pulses enable significantly greater number of hot electrons to be produced.

  7. Electron Beam Energy Compensation by Controlling RF Pulse Shape

    CERN Document Server

    Kii, T; Kusukame, K; Masuda, K; Nakai, Y; Ohgaki, H; Yamazaki, T; Yoshikawa, K; Zen, H

    2005-01-01

    We have studied on improvement of electron beam macropulse properties from a thermionic RF gun. Though a thermionic RF gun has many salient features, there is a serious problem that back-bombardment effect worsens quality of the beam. To reduce beam energy degradation by this effect, we tried to feed non-flat RF power into the gun. As a result, we successfully obtained about 1.5 times longer macropulse and two times larger total charge per macropulse. On the other hand, we calculated transient evolution of RF power considering non-constant beam loading. The beam loading is evaluated from time evolution of cathode temperature, by use of one dimensional heat conduction model and electron trajectories' calculations by a particle simulation code. Then we found good agreement between the experimental and calculation results. Furthermore, with the same way, we studied the electron beam output dependence on the cathode radius.

  8. Injection of electrons by colliding laser pulses in a laser wakefield accelerator

    CERN Document Server

    Hansson, Martin; Ekerfelt, Henrik; Persson, Anna; Lundh, Olle

    2016-01-01

    To improve the stability and reproducibility of laser wakefield accelerators and to allow for future applications, controlling the injection of electrons is of great importance. This allows us to control the amount of charge in the beams of accelerated electrons and final energy of the electrons. Results are presented from a recent experiment on controlled injection using the scheme of colliding pulses and performed using the Lund multi-terawatt laser. Each laser pulse is split into two parts close to the interaction point. The main pulse is focused on a 2 mm diameter gas jet to drive a nonlinear plasma wave below threshold for self-trapping. The second pulse, containing only a fraction of the total laser energy, is focused to collide with the main pulse in the gas jet under an angle of 150°. Beams of accelerated electrons with low divergence and small energy spread are produced using this set-up. Control over the amount of accelerated charge is achieved by rotating the plane of polarization of the second p...

  9. Review of supershort avalanche electron beam during nanosecond-pulse discharges in some gases

    Directory of Open Access Journals (Sweden)

    Victor F. Tarasenko

    2017-05-01

    Full Text Available Supershort avalanche electron beam (SAEB plays an important role in nanosecond-pulse discharges. This paper aims at reviewing experiments results on characteritics of SAEB and its spectra in different gases in nanosecond-pulse discharges. All the joint experiments were carried in the Institute of High Current Electronics of the Russian Academy of Sciences and the Institute of Electrical Engineering of the Chinese Academy of Sciences. In these experiments, the generation of a SAEB in SF6 in an inhomogeneous electric field was studied on three generators with pulse rise times of 0.3, 0.5 and ∼2 ns. Firstly, the comparison of SAEB parameters in SF6 with those obtained in other gases (air, nitrogen, argon, and krypton is introduced. Secondly, the SAEB spectra in SF6 and air at pressures of 10 kPa (75 torr, and 0.1 MPa (750 torr are reviewed and discussed. Finally, 1.5-D theoretical simulation of the supershort pulse of the fast electron beam in a coaxial diode filled with SF6 at atmospheric pressure is described. The simulation was carried out in the framework of hybrid model for discharge and runaway electron kinetics. The above research progress can provide better understanding of the investigation into the mechanism of nanosecond-pulse discharges.

  10. Microstructure Modifications and Associated Corrosion Improvements in GH4169 Superalloy Treated by High Current Pulsed Electron Beam

    OpenAIRE

    Su, Yichang; Li, Guangyu; Niu, Liyuan; Yang, Shengzhi; Cai, Jie; Guan, Qingfeng

    2015-01-01

    The surface of the nickel-based superalloy GH4169 was subjected to high-current pulsed electron beam (HCPEB) treatment. The microstructural morphologies of the material were analysed by means of optical microscope (OP), scanning electron microscope (SEM), and transmission electron microscope (TEM). The results reveal that the irradiated surface was remelted and many craters were formed. The density of craters decreased with the increment of HCPEB pulses. After 20-pulsed HCPEB irradiation, nan...

  11. Electron beam-based sources of ultrashort x-ray pulses.

    Energy Technology Data Exchange (ETDEWEB)

    Zholents, A.; Accelerator Systems Division (APS)

    2010-09-30

    A review of various methods for generation of ultrashort x-ray pulses using relativistic electron beam from conventional accelerators is presented. Both spontaneous and coherent emission of electrons is considered. The importance of the time-resolved studies of matter at picosecond (ps), femtosecond (fs), and atttosecond (as) time scales using x-rays has been widely recognized including by award of a Nobel Prize in 1999 [Zewa]. Extensive reviews of scientific drivers can be found in [BES1, BES2, BES3, Lawr, Whit]. Several laser-based techniques have been used to generate ultrashort x-ray pulses including laser-driven plasmas [Murn, Alte, Risc, Rose, Zamp], high-order harmonic generation [Schn, Rund, Wang, Arpi], and laser-driven anode sources [Ande]. In addition, ultrafast streak-camera detectors have been applied at synchrotron sources to achieve temporal resolution on the picosecond time scale [Wulf, Lind1]. In this paper, we focus on a different group of techniques that are based on the use of the relativistic electron beam produced in conventional accelerators. In the first part we review several techniques that utilize spontaneous emission of electrons and show how solitary sub-ps x-ray pulses can be obtained at existing storage ring based synchrotron light sources and linacs. In the second part we consider coherent emission of electrons in the free-electron lasers (FELs) and review several techniques for a generation of solitary sub-fs x-ray pulses. Remarkably, the x-ray pulses that can be obtained with the FELs are not only significantly shorter than the ones considered in Part 1, but also carry more photons per pulse by many orders of magnitude.

  12. Controlled injection and acceleration of electrons in plasma wakefields by colliding laser pulses.

    Science.gov (United States)

    Faure, J; Rechatin, C; Norlin, A; Lifschitz, A; Glinec, Y; Malka, V

    2006-12-07

    In laser-plasma-based accelerators, an intense laser pulse drives a large electric field (the wakefield) which accelerates particles to high energies in distances much shorter than in conventional accelerators. These high acceleration gradients, of a few hundreds of gigavolts per metre, hold the promise of compact high-energy particle accelerators. Recently, several experiments have shown that laser-plasma accelerators can produce high-quality electron beams, with quasi-monoenergetic energy distributions at the 100 MeV level. However, these beams do not have the stability and reproducibility that are required for applications. This is because the mechanism responsible for injecting electrons into the wakefield is based on highly nonlinear phenomena, and is therefore hard to control. Here we demonstrate that the injection and subsequent acceleration of electrons can be controlled by using a second laser pulse. The collision of the two laser pulses provides a pre-acceleration stage which provokes the injection of electrons into the wakefield. The experimental results show that the electron beams obtained in this manner are collimated (5 mrad divergence), monoenergetic (with energy spread electron bunch durations shorter than 10 fs. We anticipate that this stable and compact electron source will have a strong impact on applications requiring short bunches, such as the femtolysis of water, or high stability, such as radiotherapy with high-energy electrons or radiography for materials science.

  13. Laser sources for polarized electron beams in cw and pulsed accelerators

    CERN Document Server

    Hatziefremidis, A; Fraser, D; Avramopoulos, H

    1999-01-01

    We report the characterization of a high power, high repetition rate, mode-locked laser system to be used in continuous wave and pulsed electron accelerators for the generation of polarized electron beams. The system comprises of an external cavity diode laser and a harmonically mode-locked Ti:Sapphire oscillator and it can provide up to 3.4 W average power, with a corresponding pulse energy exceeding 1 nJ at 2856 MHz repetition rate. The system is tunable between 770-785 and 815-835 nm with two sets of diodes for the external cavity diode laser. (author)

  14. Paired-pulse facilitation achieved in protonic/electronic hybrid indium gallium zinc oxide synaptic transistors

    Energy Technology Data Exchange (ETDEWEB)

    Guo, Li Qiang, E-mail: guoliqiang@ujs.edu.cn; Ding, Jian Ning; Huang, Yu Kai [Micro/Nano Science & Technology Center, Jiangsu University, Zhenjiang, 212013 (China); Zhu, Li Qiang, E-mail: lqzhu@nimte.ac.cn [Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201 (China)

    2015-08-15

    Neuromorphic devices with paired pulse facilitation emulating that of biological synapses are the key to develop artificial neural networks. Here, phosphorus-doped nanogranular SiO{sub 2} electrolyte is used as gate dielectric for protonic/electronic hybrid indium gallium zinc oxide (IGZO) synaptic transistor. In such synaptic transistors, protons within the SiO{sub 2} electrolyte are deemed as neurotransmitters of biological synapses. Paired-pulse facilitation (PPF) behaviors for the analogous information were mimicked. The temperature dependent PPF behaviors were also investigated systematically. The results indicate that the protonic/electronic hybrid IGZO synaptic transistors would be promising candidates for inorganic synapses in artificial neural network applications.

  15. Paired-pulse facilitation achieved in protonic/electronic hybrid indium gallium zinc oxide synaptic transistors

    Science.gov (United States)

    Guo, Li Qiang; Zhu, Li Qiang; Ding, Jian Ning; Huang, Yu Kai

    2015-08-01

    Neuromorphic devices with paired pulse facilitation emulating that of biological synapses are the key to develop artificial neural networks. Here, phosphorus-doped nanogranular SiO2 electrolyte is used as gate dielectric for protonic/electronic hybrid indium gallium zinc oxide (IGZO) synaptic transistor. In such synaptic transistors, protons within the SiO2 electrolyte are deemed as neurotransmitters of biological synapses. Paired-pulse facilitation (PPF) behaviors for the analogous information were mimicked. The temperature dependent PPF behaviors were also investigated systematically. The results indicate that the protonic/electronic hybrid IGZO synaptic transistors would be promising candidates for inorganic synapses in artificial neural network applications.

  16. Paired-pulse facilitation achieved in protonic/electronic hybrid indium gallium zinc oxide synaptic transistors

    Directory of Open Access Journals (Sweden)

    Li Qiang Guo

    2015-08-01

    Full Text Available Neuromorphic devices with paired pulse facilitation emulating that of biological synapses are the key to develop artificial neural networks. Here, phosphorus-doped nanogranular SiO2 electrolyte is used as gate dielectric for protonic/electronic hybrid indium gallium zinc oxide (IGZO synaptic transistor. In such synaptic transistors, protons within the SiO2 electrolyte are deemed as neurotransmitters of biological synapses. Paired-pulse facilitation (PPF behaviors for the analogous information were mimicked. The temperature dependent PPF behaviors were also investigated systematically. The results indicate that the protonic/electronic hybrid IGZO synaptic transistors would be promising candidates for inorganic synapses in artificial neural network applications.

  17. In vivo imaging of a stable paramagnetic probe by pulsed-radiofrequency electron paramagnetic resonance spectroscopy

    DEFF Research Database (Denmark)

    Murugesan; Cook; Devasahayam

    1997-01-01

    Imaging of free radicals by electron paramagnetic resonance (EPR) spectroscopy using time domain acquisition as in nuclear magnetic resonance (NMR) has not been attempted because of the short spin-spin relaxation times, typically under 1 μs, of most biologically relevant paramagnetic species......, Recent advances in radiofrequency (RF) electronics have enabled the generation of pulses of the order of 10-50 ns. Such short pulses provide adequate spectral coverage for EPR studies at 300 MHz resonant frequency. Acquisition of free induction decays (FID) of paramagnetic species possessing...

  18. Ultrashort x-ray pulse generation by nonlinear Thomson scattering of a relativistic electron with an intense circularly polarized laser pulse

    Directory of Open Access Journals (Sweden)

    F. Liu

    2012-07-01

    Full Text Available The nonlinear Thomson scattering of a relativistic electron with an intense laser pulse is calculated numerically. The results show that an ultrashort x-ray pulse can be generated by an electron with an initial energy of 5 MeV propagating across a circularly polarized laser pulse with a duration of 8 femtosecond and an intensity of about 1.1×10^{21}  W/cm^{2}, when the detection direction is perpendicular to the propagation directions of both the electron and the laser beam. The optimal values of the carrier-envelop phase and the intensity of the laser pulse for the generation of a single ultrashort x-ray pulse are obtained and verified by our calculations of the radiation characteristics.

  19. Transient self-amplified Cerenkov radiation with a short pulse electron beam

    Directory of Open Access Journals (Sweden)

    B. R. Poole

    2009-08-01

    Full Text Available An analytic and numerical examination of the slow wave Cerenkov free electron maser is presented. We consider the steady-state amplifier configuration as well as operation in the self-amplified spontaneous emission (SASE regime. The linear theory is extended to include electron beams that have a parabolic radial density inhomogeneity. Closed form solutions for the dispersion relation and modal structure of the electromagnetic field are determined in this inhomogeneous case. To determine the steady-state response, a macroparticle approach is used to develop a set of coupled nonlinear ordinary differential equations for the amplitude and phase of the electromagnetic wave, which are solved in conjunction with the particle dynamical equations to determine the response when the system is driven as an amplifier with a time harmonic source. We then consider the case in which a fast rise time electron beam is injected into a dielectric loaded waveguide. In this case, radiation is generated by SASE, with the instability seeded by the leading edge of the electron beam. A pulse of radiation is produced, slipping behind the leading edge of the beam due to the disparity between the group velocity of the radiation and the beam velocity. Short pulses of microwave radiation are generated in the SASE regime and are investigated using particle-in-cell (PIC simulations. The nonlinear dynamics are significantly more complicated in the transient SASE regime when compared with the steady-state amplifier model due to the slippage of the radiation with respect to the beam. As strong self-bunching of the electron beam develops due to SASE, short pulses of superradiant emission develop with peak powers significantly larger than the predicted saturated power based on the steady-state amplifier model. As these superradiant pulses grow, their pulse length decreases and forms a series of solitonlike pulses. Comparisons between the linear theory, macroparticle model, and PIC

  20. Pulse radiolytic studies of electron transfer processes and applications to solar photochemistry. Progress report

    Energy Technology Data Exchange (ETDEWEB)

    Neta, P.

    1995-02-01

    The pulse radiolysis technique is applied to the study of electron transfer processes in a variety of chemical systems. Reactive intermediates are produced in solution by electron pulse irradiation and the kinetics of their reactions are followed by time resolved absorption spectrophotometry. Complementary experiments are carried out with excimer laser flash photolysis. These studies are concerned with mechanisms, kinetics, and thermodynamics of reactions of organic and inorganic radicals and unstable oxidation states of metal ions. Reactions are studied in both aqueous and non-aqueous solutions. The studies focus on the unique ability of pulse radiolysis to provide absolute rate constants for reactions of many inorganic radicals and organic peroxyl radicals, species that are key intermediates in many chemical processes. A special concern of this work is the study of electron transfer reactions of metalloporphyrins, which permits evaluation of these molecules as intermediates in solar energy conversion. Metalloporphyrins react with free radicals via electron transfer, involving the ligand or the metal center, or via bonding to the metal, leading to a variety of chemical species whose behavior is also investigated. The highlights of the results during the past three years are summarized below under the following sections: (a) electron transfer reactions of peroxyl radicals, concentrating on the characterization of new peroxyl radicals derived from vinyl, phenyl, other aryl, and pyridyl; (b) solvent effects on electron transfer reactions of inorganic and organic peroxyl radicals, including reactions with porphyrins, and (c) electron transfer and alkylation reactions of metalloporphyrins and other complexes.

  1. Electron-Beam Switches For A High Peak Power Sled-II Pulse Compressor

    Energy Technology Data Exchange (ETDEWEB)

    Hirshfield, Jay, L. [Yale Univ., New Haven, CT (United States)

    2015-12-02

    Omega-P demonstrated triggered electron-beam switches on the L=2 m dual-delay-line X-band pulse compressor at Naval Research Laboratory (NRL). In those experiments, with input pulses of up to 9 MW from the Omega-P/NRL X-band magnicon, output pulses having peak powers of 140-165 MW and durations of 16-20 ns were produced, with record peak power gains M of 18-20. Switch designs are described based on the successful results that should be suitable for use with the existing SLAC SLED-II delay line system, to demonstrate C=9, M=7, and n>>78%, yielding 173ns compressed pulses with peak powers up to 350MW with input of a single 50-MW.

  2. Electron acceleration by a radially polarized laser pulse during ionization of low density gases

    Directory of Open Access Journals (Sweden)

    Kunwar Pal Singh

    2011-03-01

    Full Text Available The acceleration of electrons by a radially polarized intense laser pulse has been studied. The axial electric field of the laser is responsible for electron acceleration. The axial electric field increases with decreasing laser spot size; however, the laser pulse gets defocused sooner for smaller values and the electrons do not experience high electric field for long, reducing the energy they can reach. The electron remains confined in the electric field of the laser for longer and the electron energy peaks for the normalized laser spot size nearly equal to the normalized laser intensity parameter. Electron energy peaks for initial laser phase ϕ_{0}=π due to accelerating laser phase and decreases with transverse initial position of the electrons. The energy and angle of the emittance spectrum of the electrons generated during ionization of krypton and argon at low densities have been obtained and a right choice of laser parameters has been suggested to obtain high energy quasimonoenergetic collimated electron beams. It has been found that argon is more suitable than krypton to obtain high energy electron beams due to higher ionization potential of inner shells for the former.

  3. Pulse radiolytic and electrochemical investigations of intramolecular electron transfer in carotenoporphyrins and carotenoporphyrin-quinone triads

    Energy Technology Data Exchange (ETDEWEB)

    Land, E.J.; Lexa, D.; Bensasson, R.V.; Gust, D.; Moore, T.A. Moore, A.L.; Liddell, P.A.; Nemeth, G.A.

    1987-08-27

    Thermodynamic and kinetic aspects of intramolecular electron-transfer reactions in carotenoporphyrin dyads and carotenoid-porphyrin-quinone triads have been studied by using pulse radiolysis and cyclic voltammetry. Rapid (<1 ..mu..s) electron transfer from carotenoid radical anions to attached porphyrins has been inferred. Carotenoid cations, on the other hand, do not readily accept electrons from attached porphyrins or pyropheophorbides. Electrochemical studies provide the thermodynamic basis for these observations and also allow estimation of the energetics of photoinitiated two-step electron transfer and two-step charge recombination in triad models for photosynthetic charge separation.

  4. Intense γ ray generated by refocusing laser pulse on wakefield accelerated electrons

    Science.gov (United States)

    Feng, Jie; Wang, Jinguang; Li, Yifei; Zhu, Changqing; Li, Minghua; He, Yuhang; Li, Dazhang; Wang, Weimin; Chen, Liming

    2017-09-01

    Ultrafast x/γ ray emission from the combination of laser wake-field acceleration and plasma mirror has been investigated as a promising Thomson scattering source. However, the photon energy and yield of radiation are limited to the intensity of reflected laser pulses. We use the 2D particle in cell simulation to demonstrate that a 75TW driven laser pulse can be refocused on the accelerated electron bunches through a hemispherical plasma mirror with a small f number of 0.25. The energetic electrons with the maximum energy about 350 MeV collide with the reflected laser pulse of a0 = 3.82 at the focal spot, producing high order multi-photon Thomson scattering, and resulting in the scattering spectrum which extends up to 21.2 MeV. Such a high energy γ ray source could be applied to photonuclear reaction and materials science.

  5. Femtosecond Laser Pulses Principles and Experiments

    CERN Document Server

    Rullière, Claude

    2005-01-01

    This smooth introduction for advanced undergraduates starts with the fundamentals of lasers and pulsed optics. Thus prepared, the student is introduced to short and ultrashort laser pulses, and learns how to generate, manipulate, and measure them. Spectroscopic implications are also discussed. The second edition has been completely revised and includes two new chapters on some of the most promising and fast-developing applications in ultrafast phenomena: coherent control and attosecond pulses.

  6. Observations of Infrared Radiation During Disruptions in Textor - Heat Pulses and Runaway Electrons

    NARCIS (Netherlands)

    R. Jaspers,; Grewe, T.; Finken, K.H.; KramerFlecken, A.; Cardozo, N. J. L.; Mank, G.; Waidmann, G.

    1995-01-01

    Disruptions are studied in TEXTOR using two infrared cameras. In the thermal quench phase, fast changing heat fluxes are observed, each delivering energies larger than 1 kJ/m(2) to the limiter. These bursts are correlated with an electron temperature pulse near the limiter and an increased release

  7. Pulsed laser and electron beam induced diffusion of antimony in silicon

    Energy Technology Data Exchange (ETDEWEB)

    Fogarassy, E.; Siffert, P. (Centre de Recherches Nucleaires, 67 - Strasbourg (France)); Barbier, D.; Chemisky, G.; Laugier, A. (INSA, 69 - Villeurbanne (France))

    1983-01-01

    The aim of this work is to compare the diffusion into silicon of a thin film (approximately 100 A) of deposited antimony induced either by a pulsed laser irradiation or electron beam and to interpret the different experimental behaviours as observed by Rutherford backscattering spectrometry, by using the calculated temperature distributions obtained by solving the heat flow equation for the two different annealing processes.

  8. PULSED LASER AND ELECTRON BEAM INDUCED DIFFUSION OF ANTIMONY IN SILICON

    OpenAIRE

    Fogarassy, E.; Siffert, P; Barbier, D.; Chemisky, G.; Laugier, A.

    1983-01-01

    The aim of this work is to compare the diffusion into silicon of a thin film (~ 100 Å) of deposited antimony induced either by a pulsed laser irradiation or electron beam and to interpret the different experimental behaviours as observed by Rutherford backscattering spectrometry, by using the calculated temperature distributions obtained by solving the heat flow equation for the two different annealing processes.

  9. A Technique for Temperature and Ultimate Load Calculations of Thin Targets in a Pulsed Electron Beam

    DEFF Research Database (Denmark)

    Hansen, Jørgen-Walther; Lundsager, Per

    1979-01-01

    A technique is presented for the calculation of transient temperature distributions and ultimate load of rotationally symmetric thin membranes with uniform lateral load and exposed to a pulsed electron beam from a linear accelerator. Heat transfer by conduction is considered the only transfer...

  10. Electromagnetic cascade in high-energy electron, positron, and photon interactions with intense laser pulses

    Science.gov (United States)

    Bulanov, S. S.; Schroeder, C. B.; Esarey, E.; Leemans, W. P.

    2013-06-01

    The interaction of high-energy electrons, positrons, and photons with intense laser pulses is studied in head-on collision geometry. It is shown that electrons and/or positrons undergo a cascade-type process involving multiple emissions of photons. These photons can consequently convert into electron-positron pairs. As a result charged particles quickly lose their energy developing an exponentially decaying energy distribution, which suppresses the emission of high-energy photons, thus reducing the number of electron-positron pairs being generated. Therefore, this type of interaction suppresses the development of the electromagnetic avalanche-type discharge, i.e., the exponential growth of the number of electrons, positrons, and photons does not occur in the course of interaction. The suppression will occur when three-dimensional effects can be neglected in the transverse particle orbits, i.e., for sufficiently broad laser pulses with intensities that are not too extreme. The final distributions of electrons, positrons, and photons are calculated for the case of a high-energy e-beam interacting with a counterstreaming, short intense laser pulse. The energy loss of the e-beam, which requires a self-consistent quantum description, plays an important role in this process, as well as provides a clear experimental observable for the transition from the classical to quantum regime of interaction.

  11. Electron emission from conductors subjected to intense, short-pulse electric fields

    Science.gov (United States)

    Scarpetti, R. D.; Goerz, D. A.; Bowen, P. R.; Hodgin, R. L.; Wong, K. C.; Champney, P. D'a.

    1987-06-01

    We studied electron emission from metal electrodes subjected to electric fields ranging from 0.5 to 2.5 MV/cm for pulse durations of 3 to 10 ns. We used two high-voltage pulsers for these tests; a 500 to 700 kV, 72 ohm pulser that generated a 3 ns Gaussian pulse; and a 2 MV, 60 ohm pulser that generated a 10 ns flat-top pulse with a 1-ns risetime. The high voltage levels allowed emission studies using electrode spacings of several millimeters to several centimeters. Our studies emphasized bare and anodized aluminum surface shaving surface finishes that ranged from rolled stock to machined finishes of 2 to 400 micron-in roughness. We also investigated polished stainless steel and brass. Emphasis was on first-shot performance with subsequent pulses applied to check for possible conditioning. The background pressure was typically .00005 Torr. Our studies showed that for 10 ns pulse lengths, anodized aluminum surfaces could hold off more than twice the electric field strength of bare aluminum surfaces without appreciable electron emission. Anodized surfaces performed well at 1.0 to 1.5 MV/cm, while bare surfaces emitted at 0.5 to 0.7 MV/cm. For the shorter, 3 ns pulse lengths, anodizing was less effective at improving suppression of electron emission, while surface finish became the important factor. Electrodes with surface finishes of 40 micro-in or better roughness performed well at field strengths of up to 2.4 MV/cm. The behavior of velvet cloth as an emitter was also investigated using the 3 ns pulser. We found that velvet would emit within 3 ns at field strengths approaching 100 kV/cm.

  12. Pulse-mode measurement of electron beam halo using diamond-based detector

    Directory of Open Access Journals (Sweden)

    Hideki Aoyagi

    2012-02-01

    Full Text Available Using a diamond-based detector, the electron beam halo in a high-energy accelerator can be measured with a lower detection limit than that using other instruments, such as a core monitor, a dose meter, or an optical fiber. We have successfully measured an electron beam halo using diamond-based detectors operating in the ionization mode, which were installed in the beam duct to measure the intensity of the beam halo directly. Pulse-by-pulse measurements were adopted to suppress the background noise efficiently. Feasibility tests on the diamond-based detector and beam halo monitor were performed in the beam dump area of the 8 GeV SPring-8 synchrotron booster and at the 250 MeV SPring-8 Compact SASE Source test accelerator for the SPring-8 Angstrom Compact free electron LAser (SACLA, respectively. We achieved a lower detection limit of 2×10^{3}  electrons/pulse for single-shot measurement, which corresponds to a ratio of about 10^{-6} relative to the typical charge of the beam core of 0.3 pC. We also confirmed the feasibility of the electron beam halo monitor for use as an interlock sensor to protect undulator permanent magnets used in SACLA from radiation damage.

  13. Ultrafast unequilibrium electron dynamics of aluminium interacting with an ultra-intense x-ray pulse

    Science.gov (United States)

    Gao, Cheng; Zeng, Jiaolong; Yuan, Jianmin

    2017-10-01

    Ultrafast nonequilibrium dynamics of free electrons in an ultra-intense and ultrafast x-ray pulse interacting with a solid-density aluminium is investigated by solving Fokker-Planck equation. X-ray propagation through aluminium is determined by solving a one-dimensional radiative transfer equation which is coupled with a time-dependent rate equation. Although high energy electrons are evidently nonequilibrium, they account for a small population fraction in the total free electrons. The transmission of an ultra-intense x-ray pulse through a 1 um thick solid-density aluminium sample is calculated and compared with a recent experiment, where good agreement is found and saturable absorption is evidently observed.

  14. Single-electron pulse-height spectra in thin-gap parallel-plate chambers

    CERN Document Server

    Fonte, Paulo J R; Peskov, Vladimir; Policarpo, Armando

    1999-01-01

    Single-electron pulse-height spectra were measured in 0.6 and 1.2 mm parallel-plate chambers developed for the TOF system of the ALICE /LHC-HI experiment. Mixtures of Ar with ethane, isobutane, and SF/sub 6/ were studied. The observed spectrum shows a clear peak for all gases, suggesting efficient single-electron detection in thin parallel-plate structures. The pulse-height spectrum can be described by the weighted sum of an exponential and a Polya distribution, the Polya contribution becoming more important at higher gains. Additionally, it was found that the maximum gain, above 10/sup 6/, is limited by the appearance of streamers and depends weakly on the gas composition. The suitability of each mixture for single-electron detection is also quantitatively assessed. (8 refs).

  15. Experiments on Ion Space-Charge Neutralization with Pulsed Electron Beams

    CERN Document Server

    Herleb, U

    1996-01-01

    The method of space-charge neutralization of heavy ion beams with electron beam pulses generated with electron guns incorporating ferroelectric cathodes has been experimentally investigated. Several experiments are described, the results of which prove that the intensity of selected ion beam parts with defined charge states generated in a laser ion source may be increased by one order of magnitude. For elevated charge states the intensity amplification is more significant than for low charge states. For $Al^(7+)$ ions from an aluminium target a charge enhancement by a factor of 4 has been achieved by electron beam focusing.

  16. George E. Pake Prize Lecture: Pulsed Laser Deposition and the Oxide Electronics Revolution

    Science.gov (United States)

    Venkatesan, T.

    2012-02-01

    The discovery of the Pulsed Laser Deposition (PLD) Process at Bellcore was followed by a stream of advances in the epitaxial growth of oxides and a variety of heterostructures and interfaces. Today Oxide Electronics is a fascinating field with a great deal of new Science and potential for applications. Following a discussion of these events, my talk will focus on the adventure involved in creating a new company, Neocera, and, at the same time, pushing ahead in the evolving field of oxide electronics. There, electron spin, pairing, and alignment to create superconductivity and magnetism have opened up new frontiers for research and materials development.

  17. Lateral resolution in focused electron beam-induced deposition: scaling laws for pulsed and static exposure

    Energy Technology Data Exchange (ETDEWEB)

    Szkudlarek, Aleksandra [Empa, Laboratory for Mechanics of Materials and Nanostructures, Thun (Switzerland); AGH University of Science and Technology, Department of Solid State Physics, Faculty of Physics and Applied Computer Science, Krakow (Poland); Szmyt, Wojciech; Kapusta, Czeslaw [AGH University of Science and Technology, Department of Solid State Physics, Faculty of Physics and Applied Computer Science, Krakow (Poland); Utke, Ivo [Empa, Laboratory for Mechanics of Materials and Nanostructures, Thun (Switzerland)

    2014-12-15

    In this work, we review the single-adsorbate time-dependent continuum model for focused electron beam-induced deposition (FEBID). The differential equation for the adsorption rate will be expressed by dimensionless parameters describing the contributions of adsorption, desorption, dissociation, and the surface diffusion of the precursor adsorbates. The contributions are individually presented in order to elucidate their influence during variations in the electron beam exposure time. The findings are condensed into three new scaling laws for pulsed exposure FEBID (or FEB-induced etching) relating the lateral resolution of deposits or etch pits to surface diffusion and electron beam exposure dwell time for a given adsorbate depletion state. (orig.)

  18. Dissociative multiple ionization of diatomic molecules by extreme-ultraviolet free-electron-laser pulses

    DEFF Research Database (Denmark)

    Madsen, Lars Bojer; Leth, Henriette Astrup

    2011-01-01

    Nuclear dynamics in dissociative multiple ionization processes of diatomic molecules exposed to extreme-ultraviolet free-electron-laser pulses is studied theoretically using the Monte Carlo wave packet approach. By simulated detection of the emitted electrons, the model reduces a full propagation...... of the system to propagations of the nuclear wave packet in one specific electronic charge state at a time. Suggested ionization channels can be examined, and kinetic energy release spectra for the nuclei can be calculated and compared with experiments. Double ionization of O2 is studied as an example, and good...

  19. Effect of pulse electron beam characteristics on internal friction and structural alterations in epoxy

    Energy Technology Data Exchange (ETDEWEB)

    Zaikin, Yu.A. [Al Farabi Kazakh National University, Almaty (Kazakhstan)]. E-mail: drzaykin@mail.ru; Ismailova, G.A. [Al Farabi Kazakh National University, Almaty (Kazakhstan); Al-Sheikhly, M. [University of Maryland, College Park (United States)

    2007-08-15

    Temperature dependence of internal friction is experimentally studied in epoxy irradiated by 2.5 MeV pulse electron beam to different doses. Time dependence of internal friction characteristics associated with radiation-induced processes of polymer scission and cross-linking is analyzed and discussed. Experimental data on kinetics of structural transformations in epoxy are interpreted on the base of analytical solutions of differential equations for free radical accumulation during and after irradiation subject to the pulse irradiation mode and an arbitrary effective order of radical recombination.

  20. Electron localization in fragmentation of H2 with CEP stabilized laser pulses

    Science.gov (United States)

    Kremer, Manuel; Fischer, Bettina; Rudenko, Artem; de Jesus, Vitor L. B.; Schröter, Claus Dieter; Feuerstein, Bernold; Moshammer, Robert; Ullrich, Joachim

    2009-11-01

    Fully differential data on ionization and dissociation of H2 in ultra-short (~ 6 fs), linearly polarized, intense (~ 4.1014W/cm2) laser pulses with stabilized carrier-envelope-phase (CEP) have been measured using a reaction microscope. Depending on the CEP of the laser pulses we see a clear asymmetry in the emission direction of the created protons. Contrary to earlier measurements by Kling et al. [1] we observe the highest asymmetry for kinetic energy releases (proton energy) between 0-2 eV. This excludes the electron re-collision mechanism suggested in [1] as dominant excitation channel and requires another explanation.

  1. Practical method and device for enhancing pulse contrast ratio for lasers and electron accelerators

    Science.gov (United States)

    Zhang, Shukui; Wilson, Guy

    2014-09-23

    An apparatus and method for enhancing pulse contrast ratios for drive lasers and electron accelerators. The invention comprises a mechanical dual-shutter system wherein the shutters are placed sequentially in series in a laser beam path. Each shutter of the dual shutter system has an individually operated trigger for opening and closing the shutter. As the triggers are operated individually, the delay between opening and closing first shutter and opening and closing the second shutter is variable providing for variable differential time windows and enhancement of pulse contrast ratio.

  2. Subnanosecond breakdown development in high-voltage pulse discharge: Effect of secondary electron emission

    Science.gov (United States)

    Alexandrov, A. L.; Schweigert, I. V.; Zakrevskiy, Dm. E.; Bokhan, P. A.; Gugin, P.; Lavrukhin, M.

    2017-10-01

    A subnanosecond breakdown in high-voltage pulse discharge may be a key tool for superfast commutation of high power devices. The breakdown in high-voltage open discharge at mid-high pressure in helium was studied in experiment and in kinetic simulations. The kinetic model of electron avalanche development was constructed, based on PIC-MCC simulations, including dynamics of electrons, ions and fast helium atoms, produced by ions scattering. Special attention was paid to electron emission processes from cathode, such as: photoemission by Doppler-shifted resonant photons, produced in excitation processes involving fast atoms; electron emission by ions and fast atoms bombardment of cathode; the secondary electron emission (SEE) by hot electrons from bulk plasma. The simulations show that the fast atoms accumulation is the main reason of emission growth at the early stage of breakdown, but at the final stage, when the voltage on plasma gap diminishes, namely the SEE is responsible for subnanosecond rate of current growth. It was shown that the characteristic time of the current growth can be controlled by the SEE yield. The influence of SEE yield for three types of cathode material (titanium, SiC, and CuAlMg-alloy) was tested. By changing the pulse voltage amplitude and gas pressure, the area of existence of subnanosecond breakdown is identified. It is shown that in discharge with SiC and CuAlMg-alloy cathodes (which have enhanced SEE) the current can increase with a subnanosecond characteristic time value as small as τs = 0.4 ns, for the pulse voltage amplitude of 5÷12 kV. An increase of gas pressure from 15 Torr to 30 Torr essentially decreases the time of of current front growth, whereas the pulse voltage variation weakly affects the results.

  3. Attosecond relative delay among xenon 5p, 5s, and 4d photoionization

    Science.gov (United States)

    Magrakvelidze, Maia; Madjet, Mohamed; Chakraborty, Himadri

    2017-04-01

    Attosecond Wigner-Smith (WS) time delays of the photoemissions of Xe valence 5p, 5s, and core 4d electrons are investigated in details using the time-dependent local density approximation (TDLDA). Electron correlations determine the energy-dependent structures in ionization phases of the dipole channels and in the resulting WS delays at various shape resonances, induced by the collective motion of 4d electrons, and at various Cooper minima. We find that our calculation closely agrees with the streaking measurement for the delay of 4d relative to 5s, and predicts accelerated emission of 5p with respect to 4d as was experimentally observed at similar photon energies for Xe atoms adsorbed on the tungsten surface. This work was supported by the U.S. National Science Foundation.

  4. Multi-pulsed intense electron beam emission from velvet, carbon fibers, carbon nano-tubes and dispenser cathodes

    Science.gov (United States)

    Xia, Lian-Sheng; Yang, An-Min; Chen, Yi; Zhang, Huang; Liu, Xing-Guang; Li, Jin; Jiang, Xiao-Guo; Zhang, Kai-Zhi; Shi, Jin-Shui; Deng, Jian-Jun; Zhang, Lin-Wen

    2010-11-01

    The experimental results of studies of four kinds of cathode emitting intense electron beams are demonstrated under multi-pulsed mode based on an experimental setup including two multi-pulse high voltage sources. The tested cathodes include velvet, carbon fibers, carbon nano-tubes (CNTs) and dispenser cathodes. The results indicate that all four are able to emit multi-pulsed beams. For velvet, carbon fiber and CNTs, the electron induced cathode plasma emission may be the main process and this means that there are differences in beam parameters from pulse to pulse. For dispenser cathodes tested in the experiment, although there is a little difference from pulse to pulse for some reason, thermal-electric field emission may be the main process.

  5. Pulse shape optimization for electron-positron production in rotating fields

    Science.gov (United States)

    Fillion-Gourdeau, François; Hebenstreit, Florian; Gagnon, Denis; MacLean, Steve

    2017-07-01

    We optimize the pulse shape and polarization of time-dependent electric fields to maximize the production of electron-positron pairs via strong field quantum electrodynamics processes. The pulse is parametrized in Fourier space by a B -spline polynomial basis, which results in a relatively low-dimensional parameter space while still allowing for a large number of electric field modes. The optimization is performed by using a parallel implementation of the differential evolution, one of the most efficient metaheuristic algorithms. The computational performance of the numerical method and the results on pair production are compared with a local multistart optimization algorithm. These techniques allow us to determine the pulse shape and field polarization that maximize the number of produced pairs in computationally accessible regimes.

  6. Nanofocusing of hard X-ray free electron laser pulses using diamond based Fresnel zone plates

    Science.gov (United States)

    David, C.; Gorelick, S.; Rutishauser, S.; Krzywinski, J.; Vila-Comamala, J.; Guzenko, V. A.; Bunk, O.; Färm, E.; Ritala, M.; Cammarata, M.; Fritz, D. M.; Barrett, R.; Samoylova, L.; Grünert, J.; Sinn, H.

    2011-08-01

    A growing number of X-ray sources based on the free-electron laser (XFEL) principle are presently under construction or have recently started operation. The intense, ultrashort pulses of these sources will enable new insights in many different fields of science. A key problem is to provide x-ray optical elements capable of collecting the largest possible fraction of the radiation and to focus into the smallest possible focus. As a key step towards this goal, we demonstrate here the first nanofocusing of hard XFEL pulses. We developed diamond based Fresnel zone plates capable of withstanding the full beam of the world's most powerful x-ray laser. Using an imprint technique, we measured the focal spot size, which was limited to 320 nm FWHM by the spectral band width of the source. A peak power density in the focal spot of 4×1017 W/cm2 was obtained at 70 fs pulse length.

  7. Time-resolved microplasma electron dynamics in a pulsed microwave discharge

    Science.gov (United States)

    Monfared, S. K.; Hoskinson, A. R.; Hopwood, J.

    2013-10-01

    Microwave-driven microplasmas are typically operated in a steady-state mode in which the electron temperature is constant in time. Transient measurements of excitation temperature and helium emission lines, however, suggest that short microwave pulses can be used to increase the electron energy by 20-30%. Time-resolved optical emission spectrometry reveals an initial burst of light emission from the igniting microplasma. This emission overshoot is also correlated with a measured increase in excitation temperature. Excimer emission lags atomic emission, however, and does not overshoot. A simple model shows that an increase in electron temperature is responsible for the overshoot of atomic optical emission at the beginning of each microwave pulse. The formation of dimers and subsequent excimer emission requires slower three-body collisions with the excited rare gas atoms, which is why excimer emission does not overshoot the steady-state values. Similar results are observed in argon gas. The overshoot in electron temperature may be used to manipulate the collisional production of species in microplasmas using short, low-duty cycle microwave pulses.

  8. Modeling of beam-target interaction during pulsed electron beam ablation of graphite: Case of melting

    Energy Technology Data Exchange (ETDEWEB)

    Ali, Muddassir, E-mail: mx1_ali@laurentian.ca; Henda, Redhouane

    2017-02-28

    Highlights: • Modeling of ablation stage induced during pulsed electron beam ablation (PEBA). • Thermal model to describe heating, melting and vaporization of a graphite target. • Model results show good accordance with reported data in the literature. - Abstract: A one-dimensional thermal model based on a two-stage heat conduction equation is employed to investigate the ablation of graphite target during nanosecond pulsed electron beam ablation. This comprehensive model accounts for the complex physical phenomena comprised of target heating, melting and vaporization upon irradiation with a polyenergetic electron beam. Melting and vaporization effects induced during ablation are taken into account by introducing moving phase boundaries. Phase transition induced during ablation is considered through the temperature dependent thermodynamic properties of graphite. The effect of electron beam efficiency, power density, and accelerating voltage on ablation is analyzed. For an electron beam operating at an accelerating voltage of 15 kV and efficiency of 0.6, the model findings show that the target surface temperature can reach up to 7500 K at the end of the pulse. The surface begins to melt within 25 ns from the pulse start. For the same process conditions, the estimated ablation depth and ablated mass per unit area are about 0.60 μm and 1.05 μg/mm{sup 2}, respectively. Model results indicate that ablation takes place primarily in the regime of normal vaporization from the surface. The results obtained at an accelerating voltage of 15 kV and efficiency factor of 0.6 are satisfactorily in good accordance with available experimental data in the literature.

  9. Ultrafast dynamics driven by intense light pulses from atoms to solids, from lasers to intense X-rays

    CERN Document Server

    Gräfe, Stefanie

    2016-01-01

    This book documents the recent vivid developments in the research field of ultrashort intense light pulses for probing and controlling ultrafast dynamics. The recent fascinating results in studying and controlling ultrafast dynamics in ever more complicated systems such as (bio-)molecules and structures of meso- to macroscopic sizes on ever shorter time-scales are presented. The book is written by some of the most eminent experimental and theoretical experts in the field. It covers the new groundbreaking research directions that were opened by the availability of new light sources such as fully controlled intense laser fields with durations down to a single oscillation cycle, short-wavelength laser-driven attosecond pulses and intense X-ray pulses from the upcoming free electron lasers. These light sources allowed the investigation of dynamics in atoms, molecules, clusters, on surfaces and very recently also in nanostructures and solids in new regimes of parameters which, in turn, led to the identification of...

  10. Electron heating by intense short-pulse lasers propagating through near-critical plasmas

    Science.gov (United States)

    Debayle, A.; Mollica, F.; Vauzour, B.; Wan, Y.; Flacco, A.; Malka, V.; Davoine, X.; Gremillet, L.

    2017-12-01

    We investigate the electron heating induced by a relativistic-intensity laser pulse propagating through a near-critical plasma. Using particle-in-cell simulations, we show that a specific interaction regime sets in when, due to the energy depletion caused by the plasma wakefield, the laser front profile has steepened to the point of having a length scale close to the laser wavelength. Wave breaking and phase mixing have then occurred, giving rise to a relativistically hot electron population following the laser pulse. This hot electron flow is dense enough to neutralize the cold bulk electrons during their backward acceleration by the wakefield. This neutralization mechanism delays, but does not prevent the breaking of the wakefield: the resulting phase mixing converts the large kinetic energy of the backward-flowing electrons into thermal energy greatly exceeding the conventional ponderomotive scaling at laser intensities > {10}21 {{{W}}{cm}}-2 and gas densities around 10% of the critical density. We develop a semi-numerical model, based on the Akhiezer–Polovin equations, which correctly reproduces the particle-in-cell-predicted electron thermal energies over a broad parameter range. Given this good agreement, we propose a criterion for full laser absorption that includes field-induced ionization. Finally, we show that our predictions still hold in a two-dimensional geometry using a realistic gas profile.

  11. Pulse duration and wavelength stability measurements of a midinfrared free-electron laser.

    Science.gov (United States)

    Qin, Yu; Zen, Heishun; Wang, Xiaolong; Kii, Toshiteru; Nakajima, Takashi; Ohgaki, Hideaki

    2013-04-01

    We report the pulse duration and wavelength stability measurements of a midinfrared free-electron laser (FEL) where the wavelength fluctuation may not be negligible. The technique we employ is a fringe-resolved autocorrelation (FRAC) method that has good sensitivity on not only the pulse duration and the chirp but also the wavelength stability. By the simple manipulation of experimental FRAC signals, we can obtain the pulse duration even if the amounts of the chirp and the wavelength stability are not known in advance, which is further used to estimate the wavelength stability. Through this procedure we find that the pulse duration of the Kyoto University FEL at 12 μm is about 0.58 ps without any notable chirp, and the wavelength stability is about 1.3%. We also carry out separate experiments for intensity autocorrelation and sum-frequency mixing. The difference we find for pulse duration and wavelength stability by the different measurements is attributed to the different operation conditions of FEL.

  12. The microstructures and corrosion properties of polycrystalline copper induced by high-current pulsed electron beam

    Science.gov (United States)

    Zhang, Zaiqiang; Yang, Shengzhi; Lv, Peng; Li, Yan; Wang, Xiaotong; Hou, Xiuli; Guan, Qingfeng

    2014-03-01

    In order to investigate the corrosion mechanism of pure metal materials containing little impurities, polycrystalline commercial pure (cp) copper was irradiated by high-current pulsed electron beam (HCPEB). The surface microstructures of irradiated samples are characterized by using optical microscopy and transmission electron microscopy (TEM). The corrosion resistance is also investigated by using polarization curves of seawater corrosion and electrode impedance spectroscopy (EIS). The experimental results indicate that the corrosion resistance of cp copper irradiated by 10 pulses is remarkably improved comparing with the original sample. TEM observations suggest that large amount of supersaturated vacancy defects are produced when the material surface is subjected to the HCPEB irradiation. Furthermore, the agglomerations of the vacancy defects cause the formation of the vacancy cluster defects, such as vacancy dislocation loops, the stacking fault tetrahedra (SFTs) and voids. It is suggested that the structural defects on the irradiated surface have some relationships with the corrosion resistance's improvement of the material.

  13. Power pulsing scheme for analog and digital electronics of the vertex detectors at CLIC

    CERN Document Server

    Blanchot, Georges

    2015-01-01

    The precision requirements of the vertex detector at CLIC impose strong limitations on the mass of such a detector (< 0.2% of a radiation length, Xo, per layer). To achieve such a low material budget, ultra-thin hybrid pixel detectors are foreseen, while the mass for cooling and services will be reduced by implementing a power pulsing scheme that takes advantage of the low duty cycle of the accelerator. The principal aim is to achieve significant power reduction without compromising the power integrity supplied to the front-end electronics. This report summarises the study of a power pulsing scheme to power the vertex barrel electronics of the future CLIC experiment. Its main goal is to describe in more detail what has been already presented in TWEPP conferences and other presentations. The report can therefore serve as an operator manual for future use and development of the system

  14. Enhancement of ultrafast electron photoemission from metallic nano antennas excited by a femtosecond laser pulse

    CERN Document Server

    Gubko, M A; Ionin, A A; Kudryashov, S I; Makarov, S V; Nathala, C S R; Rudenko, A A; Seleznev, L V; Sinitsyn, D V; Treshin, I V

    2013-01-01

    We have demonstrated for the first time that an array of nanoantennas (central nanotips inside sub-micron pits) on an aluminum surface, fabricated using a specific double-pulse femtosecond laser irradiation scheme, results in a 28-fold enhancement of the non-linear (three-photon) electron photoemission yield, driven by a third intense IR femtosecond laser pulse. The supporting numerical electrodynamic modeling indicates that the electron emission is increased not owing to a larger effective aluminum surface, but due to instant local electromagnetic field enhancement near the nanoantenna, contributed by both the tip's lightning rod effect and the focusing effect of the pit as a microreflector and annular edge as a plasmonic lens.

  15. Reflection of femtosecond pulses from soft X-ray free-electron laser by periodical multilayers

    Energy Technology Data Exchange (ETDEWEB)

    Ksenzov, D.; Grigorian, S.; Pietsch, U. [Faculty of Physics, University of Siegen (Germany); Hendel, S.; Bienert, F.; Sacher, M.D.; Heinzmann, U. [Faculty of Physics, University of Bielefeld (Germany)

    2009-08-15

    Recent experiments on a soft X-ray free-electron laser (FEL) source (FLASH in Hamburg) have shown that multilayers (MLs) can be used as optical elements for highly intense X-ray irradiation. An effort to find most appropriate MLs has to consider the femtosecond time structure and the particular photon energy of the FEL. In this paper we have analysed the time response of 'low absorbing' MLs (e.g. such as La/B{sub 4}C) as a function of the number of periods. Interaction of a pulse train of Gaussian shaped sub-pulses using a realistic ML grown by electron-beam evaporation technique has been analysed in the soft-X-ray range. The structural parameters of the MLs were obtained by reflectivity measurements at BESSY II and subsequent profile fittings. (Abstract Copyright [2009], Wiley Periodicals, Inc.)

  16. Simulated electronic heterodyne recording and processing of pulsed-laser holograms

    Science.gov (United States)

    Decker, A. J.

    1979-01-01

    The electronic recording of pulsed-laser holograms is proposed. The polarization sensitivity of each resolution element of the detector is controlled independently to add an arbitrary phase to the image waves. This method which can be used to simulate heterodyne recording and to process three-dimensional optical images, is based on a similar method for heterodyne recording and processing of continuous-wave holograms.

  17. The effect of electron transport on the characterization of x-ray free-electron laser pulses via ablation

    Science.gov (United States)

    Hau-Riege, Stefan P.; Pardini, Tom

    2017-10-01

    The spatial intensity distribution of x-ray free-electron laser (XFEL) pulses in-focus is commonly characterized by performing ablative imprints in thin gold films on silica substrates. In many cases, the range of the electrons generated in the gold by x-ray absorption far exceeds the beam size, and so, it is not clear if the results of imprint studies are compromised by electron transport. Thermal conduction could further modify the energy density profile in the material. We used a combination of Monte-Carlo transport and continuum models to quantify the accuracy of the imprint method for characterizing XFEL beam profiles. We found that for x-ray energies in the range of 1 to 10 keV, the actual and the measured beam diameters agree within 12% or better for beam diameters between 0.1 and 1 μm.

  18. Pinched propagation of high-power, pulsed electron beams for welding and materials processing applications

    Science.gov (United States)

    Fernsler, Richard F.; Hubbard, Richard F.; Lampe, Martin

    1994-01-01

    Electron beams are used commercially as intense heating sources for welding and related materials processing applications. The beams used for welding operate continuously with energy up to 200 keV and current approximately 1 A. Because these beams are severely degraded by propagation in air over any substantial range, most present-day electron-beam welders require vacuum pumping and precision focusing, which has severely restricted utilization of the technology. Over the past few decades, a different class of electron-beam generators has been developed that produces pulsed beams with energies of several MeV, currents of 1 kA or more, radii as small as 1 mm, pulse lengths of tens of ns, and pulse repetition rates up to several kHz. We show here that beams of this type can propagate in ambient air, in a tightly pinched mode and with acceptable stability, over distances of a few tens of cm. We determine the constraints on the choice of beam parameters, due mainly to the effects of gas scattering and the resistive instability. We show that stability can be enhanced, and the acceptable parameter range extended considerably, by using a narrow conducting pipe filled with air or another gas to guide the beam to the workpiece.

  19. Microstructures and properties of zirconium-702 irradiated by high current pulsed electron beam

    Science.gov (United States)

    Yang, Shen; Cai, Jie; Lv, Peng; Zhang, Conglin; Huang, Wei; Guan, Qingfeng

    2015-09-01

    The microstructure, hardness and corrosion resistance of zirconium-702 before and after high-current pulsed electron beam (HCPEB) irradiation have been investigated. The microstructure evolution and surface morphologies of the samples were characterized by using X-ray diffraction (XRD), optical microscopy (OM), scanning electron microscopy (SEM), and transmission electron microscopy (TEM). The experimental results indicate that the sample surface was melted after HCPEB irradiation, and martensitic phase transformation occurred. Besides, two kinds of craters as well as ultrafine structures were obtained in the melted layer. TEM observations suggest that high density dislocations and deformation twins were formed after HCPEB irradiation. With the increasing of pulses, microhardness of the irradiated samples was increased from the initial 178 Hv to 254 Hv. The corrosion resistance was tested by using electrode impedance spectroscopy (EIS) and potentiodynamic polarization curves. Electrochemical results show that, after HCPEB irradiation, all the samples had better corrosion resistance in 1 mol HNO3 solution compared to the initial one, among which the 5-pulsed sample owned the best corrosion resistance. Ultrafine structures, martensitic phase transformation, surface porosities, dislocations and deformation twins are believed to be the dominant reasons for the improvement of the hardness and corrosion resistance.

  20. Review of high-power pulsed systems at the Institute of High Current Electronics

    Directory of Open Access Journals (Sweden)

    A.A. Kim

    2016-07-01

    Full Text Available In this paper, we give a review of some most powerful pulsed systems developed at the Institute of High Current Electronics (HCEI, Siberian Branch, Russian Academy of Sciences, and describe latest achievements of the teams dealing with these installations. Besides the presented high-power systems, HCEI performs numerous investigations using much less powerful generators. For instance, last year much attention was paying to the research and development of the intense low-energy (<200 kV high-current electron and ion beam and plasma sources, and their application in the technology [1–3].

  1. Strongly directed electron emission in non-sequential double ionization of Ne by intense laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Moshammer, R [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, D-67119 Heidelberg (Germany); Ullrich, J [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, D-67119 Heidelberg (Germany); Feuerstein, B [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, D-67119 Heidelberg (Germany); Fischer, D [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, D-67119 Heidelberg (Germany); Dorn, A [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, D-67119 Heidelberg (Germany); Schroeter, C D [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, D-67119 Heidelberg (Germany); Lopez-Urrutia, J R Crespo [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, D-67119 Heidelberg (Germany); Hoehr, C [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, D-67119 Heidelberg (Germany); Rottke, H [Max-Born-Institut, Max-Born-Strasse 2a, D-12489 Berlin (Germany); Trump, C [Max-Born-Institut, Max-Born-Strasse 2a, D-12489 Berlin (Germany); Wittmann, M [Max-Born-Institut, Max-Born-Strasse 2a, D-12489 Berlin (Germany); Korn, G [Max-Born-Institut, Max-Born-Strasse 2a, D-12489 Berlin (Germany); Hoffmann, K [Max-Born-Institut, Max-Born-Strasse 2a, D-12489 Berlin (Germany); Sandner, W [Max-Born-Institut, Max-Born-Strasse 2a, D-12489 Berlin (Germany)

    2003-03-28

    Double ionization of Ne by 25 fs, 1.0 PW cm{sup -2} laser pulses has been explored in a kinematically complete experiment using a 'reaction microscope'. Electrons are found to be emitted into a narrow cone along the laser polarization ({epsilon}), much more confined than for single ionization, with a broad maximum in their energy distribution along {epsilon}. Correlated momentum spectra show both electrons being ejected into the same hemisphere, in sharp contrast to predictions based on field-free (e, 2e) recollision dynamics, but in overall agreement with recent semiclassical calculations for He. (letter to the editor)

  2. Ultrafast electron field emission from gold resonant antennas studied by two terahertz pulse experiments

    DEFF Research Database (Denmark)

    Iwaszczuk, Krzysztof; Zalkovskij, Maksim; Strikwerda, Andrew C.

    2015-01-01

    Summary form only given. Ultrafast electron field emission from gold resonant antennas induced by strong terahertz (THz) transient is investigated using two THz pulse experiments. It is shown that UV emission from nitrogen plasma generated by liberated electrons is a good indication of the local...... electric field at the antenna tip. Using this method resonant properties of antennas fabricated on high resistivity silicon are investigated in the strong field regime. Decrease of antenna Q-factor due to ultrafast carrier multiplication in the substrate is observed....

  3. Modal description of longitudinal space-charge fields in pulse-driven free-electron devices

    Directory of Open Access Journals (Sweden)

    Yu. Lurie

    2010-05-01

    Full Text Available In pulsed-beam free-electron devices, longitudinal space-charge fields result in collective effects leading to an expansion of short electron bunches along their trajectory. This effect restricts an application of intense ultrashort electron pulses in free-electron radiation sources. A careful theoretical treatment is required in order to achieve an accurate description of the self-fields and the resulted electron beam dynamics. In this paper, longitudinal space-charge fields are considered in the framework of a three-dimensional, space-frequency approach. The model is based on the expansion of the total electromagnetic field (including self-fields in terms of transverse eigenmodes of the (cold cavity, in which the field is excited and propagates. The electromagnetic field, originally obtained in the model as a solution of the wave equation, is shown to satisfy also Gauss’s law. We applied the theory to derive an analytical expression for the longitudinal electric field of a pointlike charge, moving along a waveguide at a constant velocity. This enables consideration and study of the role played by different terms of the resulted expressions, such as components arising from forward and backward waves, propagating waves, and under cutoff frequencies, and so on. Possible simplifications in evaluation of longitudinal space-charge fields are discussed.

  4. High-energy-density electron beam from interaction of two successive laser pulses with subcritical-density plasma

    Directory of Open Access Journals (Sweden)

    J. W. Wang

    2016-02-01

    Full Text Available It is shown by particle-in-cell simulations that a narrow electron beam with high energy and charge density can be generated in a subcritical-density plasma by two consecutive laser pulses. Although the first laser pulse dissipates rapidly, the second pulse can propagate for a long distance in the thin wake channel created by the first pulse and can further accelerate the preaccelerated electrons therein. Given that the second pulse also self-focuses, the resulting electron beam has a narrow waist and high charge and energy densities. Such beams are useful for enhancing the target-back space-charge field in target normal sheath acceleration of ions and bremsstrahlung sources, among others.

  5. Scanning electron microscopy and ablation rates of hard dental tissue using 350-fs and 1-ns laser pulses

    Science.gov (United States)

    Neev, Joseph; Huynh, Daniel S.; Dan, Claudiu C.; White, Joel M.; Da Silva, Luiz B.; Feit, Michael D.; Matthews, Dennis L.; Perry, Michael D.; Rubenchik, Alexander M.; Stuart, Brent C.

    1996-04-01

    Lasers are currently limited in their ability to remove hard tissue. Furthermore, many laser systems, such as the long pulse infrared lasers used to ablate bone or hard dental tissue, also generate unacceptable heat levels and cause collateral tissue damage. Ultrashort pulse lasers, however, are highly efficient, quiet, and relatively free of charge. With recent developments now allowing operation at high pulse repetition rates, ultrashort pulse systems can yield significant material volume removal which can potentially match or even exceed conventional technology while still maintaining the minimal collateral damage characteristics. In this paper, the interaction characteristics of two pulse regimes with enamel and dentin: 350 fs pulse ablation of hard dental tissues is compared to the interaction with one nanosecond pulses. Ablation rates were characterized and surface morphology, and structure were evaluated using a scanning electron microscope.

  6. Tracing the phase of focused broadband laser pulses

    Science.gov (United States)

    Hoff, Dominik; Krüger, Michael; Maisenbacher, Lothar; Sayler, A. M.; Paulus, Gerhard G.; Hommelhoff, Peter

    2017-10-01

    Precise knowledge of the behaviour of the phase of light in a focused beam is fundamental to understanding and controlling laser-driven processes. More than a hundred years ago, an axial phase anomaly for focused monochromatic light beams was discovered and is now commonly known as the Gouy phase. Recent theoretical work has brought into question the validity of applying this monochromatic phase formulation to the broadband pulses becoming ubiquitous today. Based on electron backscattering at sharp nanometre-scale metal tips, a method is available to measure light fields with sub-wavelength spatial resolution and sub-optical-cycle time resolution. Here we report such a direct, three-dimensional measurement of the spatial dependence of the optical phase of a focused, 4-fs, near-infrared pulsed laser beam. The observed optical phase deviates substantially from the monochromatic Gouy phase--exhibiting a much more complex spatial dependence, both along the propagation axis and in the radial direction. In our measurements, these significant deviations are the rule and not the exception for focused, broadband laser pulses. Therefore, we expect wide ramifications for all broadband laser-matter interactions, such as in high-harmonic and attosecond pulse generation, femtochemistry, ophthalmological optical coherence tomography and light-wave electronics.

  7. Terahertz-pulse driven modulation of electronic spectra: Modeling electron-phonon coupling in charge-transfer crystals

    Science.gov (United States)

    Di Maiolo, Francesco; Masino, Matteo; Painelli, Anna

    2017-08-01

    We calculate the optical spectra of a charge-transfer crystal modulated by a terahertz pulse, accounting for electron-vibration coupling. The model Hamiltonian is parametrized against first principle calculations and adiabatic results are validated against a fully non-adiabatic calculation where relaxation phenomena are introduced via the coupling of the quantum system to a dissipative bath of classic anharmonic oscillators. The experiment is well reproduced by the proposed model with no need to introduce any ad hoc assumption on the temporal dependence of model parameters, but just accounting for the quadratic dependence of the Hubbard U on non-totally symmetric molecular coordinates.

  8. Electron kinetic effects in atmosphere breakdown by an intense electromagnetic pulse.

    Science.gov (United States)

    Solovyev, A A; Terekhin, V A; Tikhonchuk, V T; Altgilbers, L L

    1999-12-01

    A physical model is proposed for description of electron kinetics driven by a powerful electromagnetic pulse in the Earth's atmosphere. The model is based on a numerical solution to the Boltzmann kinetic equation for two groups of electrons. Slow electrons (with energies below a few keV) are described in a two-term approximation assuming a weak anisotropy of the electron distribution function. Fast electrons (with energies above a few keV) are described by a modified macroparticle method, taking into account the electron acceleration in the electric field, energy losses in the continuous deceleration approximation, and the multiple pitch angle scattering. The model is applied to a problem of the electric discharge in a nitrogen, which is preionized by an external gamma-ray source. It is shown that the runaway electrons have an important effect on the energy distribution of free electrons, and on the avalanche ionization rate. This mechanism might explain the observation of multiple lightning discharges observed in the Ivy-Mike thermonuclear test in the early 1950's.

  9. Differences between intra- and extra-cavity pulse time structure in a hole-coupled free-electron laser

    NARCIS (Netherlands)

    Weits, H. H.; Knippels, G.M.H.; van Werkhoven, G. H. C.; Oepts, D.; van Amersfoort, P. W.

    1997-01-01

    In the strong-slippage regime of a free-electron laser, the optical pulse inside the resonator is composed of a series of subsequently growing and decaying subpulses due to a limit-cycle oscillation. The picosecond time structure of the outcoupled pulses can be quite different from that of the

  10. Effect of secondary electron emission on subnanosecond breakdown in high-voltage pulse discharge

    Science.gov (United States)

    Schweigert, I. V.; Alexandrov, A. L.; Gugin, P.; Lavrukhin, M.; Bokhan, P. A.; Zakrevsky, Dm E.

    2017-11-01

    The subnanosecond breakdown in open discharge may be applied for producing superfast high power switches. Such fast breakdown in high-voltage pulse discharge in helium was explored both in experiment and in kinetic simulations. The kinetic model of electron avalanche development was developed using PIC-MCC technique. The model simulates motion of electrons, ions and fast helium atoms, appearing due to ions scattering. It was shown that the mechanism responsible for ultra-fast breakdown development is the electron emission from cathode. The photoemission and emission by ions or fast atoms impact is the main reason of current growth at the early stage of breakdown, but at the final stage, when the voltage on discharge gap drops, the secondary electron emission (SEE) is responsible for subnanosecond time scale of current growth. It was also found that the characteristic time of the current growth τS depends on the SEE yield of the cathode material. Three types of cathode material (titanium, SiC, and CuAlMg-alloy) were tested. It is shown that in discharge with SiC and CuAlMg-alloy cathodes (which have enhanced SEE) the current can increase with a subnanosecond characteristic time as small as τS = 0.4 ns, for the pulse voltage amplitude of 5- 12 kV..

  11. Nonlinear currents generated in plasma by a radiation pulse with a frequency exceeding the electron plasma frequency

    Energy Technology Data Exchange (ETDEWEB)

    Grishkov, V. E.; Uryupin, S. A., E-mail: uryupin@sci.lebedev.ru [Russian Academy of Sciences, Lebedev Physical Institute (Russian Federation)

    2016-09-15

    It is shown that the nonlinear currents generated in plasma by a radiation pulse with a frequency exceeding the electron plasma frequency change substantially due to a reduction in the effective electron–ion collision frequency.

  12. Mapping the Dissociative Ionization Dynamics of Molecular Nitrogen with Attosecond Time Resolution

    Directory of Open Access Journals (Sweden)

    A. Trabattoni

    2015-12-01

    Full Text Available Studying the interaction of molecular nitrogen with extreme ultraviolet (XUV radiation is of prime importance to understand radiation-induced processes occurring in Earth’s upper atmosphere. In particular, photoinduced dissociation dynamics involving excited states of N_{2}^{+} leads to N and N^{+} atomic species that are relevant in atmospheric photochemical processes. However, tracking the relaxation dynamics of highly excited states of N_{2}^{+} is difficult to achieve, and its theoretical modeling is notoriously complex. Here, we report on an experimental and theoretical investigation of the dissociation dynamics of N_{2}^{+} induced by isolated attosecond XUV pulses in combination with few-optical-cycle near-infrared/visible (NIR/VIS pulses. The momentum distribution of the produced N^{+} fragments is measured as a function of pump-probe delay with subfemtosecond resolution using a velocity map imaging spectrometer. The time-dependent measurements reveal the presence of NIR/VIS-induced transitions between N_{2}^{+} states together with an interference pattern that carries the signature of the potential energy curves activated by the XUV pulse. We show that the subfemtosecond characterization of the interference pattern is essential for a semiquantitative determination of the repulsive part of these curves.

  13. A Method to Determine Diastolic Blood Pressure Based on Pressure Pulse Propagation in the Electronic Palpation Method

    Science.gov (United States)

    2001-10-25

    electronically palpated pulse. This particular patient seems to have arrhythmia, and, because of that, oscillometric blood pressure methods may give...of multiple oscillometric methods for blood pressure measurement in finger�, Proceedings of The First Joint BMES/EMBS Conference Serving Humanity...1 of 4 A METHOD TO DETERMINE DIASTOLIC BLOOD PRESSURE BASED ON PRESSURE PULSE PROPAGATION IN THE ELECTRONIC PALPATION METHOD H. S. S

  14. Pulse shape and spectrum of coherent diffraction-limited transition radiation from electron beams

    Energy Technology Data Exchange (ETDEWEB)

    van Tilborg, J.; Schroeder, C.B.; Esarey, E.; Leemans, W.P.

    2003-12-20

    The electric field in the temporal and spectral domain of coherent diffraction-limited transition radiation is studied. An electron bunch, with arbitrary longitudinal momentum distribution, propagating at normal incidence to a sharp metal-vacuum boundary with finite transverse dimension is considered. A general expression for the spatiotemporal electric field of the transition radiation is derived, and closed-form solutions for several special cases are given. The influence of parameters such as radial boundary size, electron momentum distribution, and angle of observation on the waveform (e.g., radiation pulse length and amplitude) are discussed. For a Gaussian electron bunch, the coherent radiation waveform is shown to have a single-cycle profile. Application to a novel THz source based on a laser-driven accelerator is discussed.

  15. Femtosecond pulsed laser processing of electronic materials: Fundamentals and micro/nano-scale applications

    Science.gov (United States)

    Choi, Tae-Youl

    Ultra-short pulsed laser radiation has been shown to be effective for precision materials processing and surface micro-modification. One of advantages is the substantial reduction of the heat penetration depth, which leads to minimal lateral damage. Other advantages include non-thermal nature of ablation process, controlled ablation and ideal characteristics for precision micro-structuring. Yet, fundamental questions remain unsolved regarding the nature of melting and ablation mechanisms in femtosecond laser processing of materials. In addition to micro engineering problems, nano-structuring and nano-fabrication are emerging fields that are of particular interest in conjunction with femtosecond laser processing. A comprehensive experimental study as well as theoretical development is presented to address these issues. Ultra-short pulsed laser irradiation was used to crystallize 100 nm amorphous silicon (a-Si) films. The crystallization process was observed by time-resolved pump-and-probe reflection imaging in the range of 0.2 ps to 100 ns. The in-situ images in conjunction with post-processed SEM and AFM mapping of the crystallized structure provide evidence for non-thermal ultra-fast phase transition and subsequent surface-initiated crystallization. Mechanisms of ultra-fast laser-induced ablation on crystalline silicon and copper are investigated by time-resolved pump-and-probe microscopy in normal imaging and shadowgraph arrangements. A one-dimensional model of the energy transport is utilized to predict the carrier temperature and lattice temperature as well as the electron and vapor flux emitted from the surface. The temporal delay between the pump and probe pulses was set by a precision translation stage up to about 500 ps and then extended to the nanosecond regime by an optical fiber assembly. The ejection of material was observed at several picoseconds to tens of nanoseconds after the main (pump) pulse by high-resolution, ultra-fast shadowgraphs. The

  16. Electron localization in fragmentation of H{sub 2} with CEP stabilized laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Kremer, Manuel; Fischer, Bettina; Schroeter, Claus Dieter; Feuerstein, Bernold; Moshammer, Robert; Ullrich, Joachim [Max-Planck-Institut fuer Kernphysik, 69117 Heidelberg (Germany); Rudenko, Artem [Max-Planck Advanced Study Group at CFEL, 22607 Hamburg (Germany); Jesus, Vitor L B de, E-mail: kremer@mpi-hd.mpg.d [Instituto Federal do Rio de Janeiro - IFRJ, 26530-060 Nilopolis-RJ (Brazil)

    2009-11-01

    Fully differential data on ionization and dissociation of H{sub 2} in ultra-short ({approx} 6 fs), linearly polarized, intense ({approx} 4{sup .}10{sup 14}W/cm{sup 2}) laser pulses with stabilized carrier-envelope-phase (CEP) have been measured using a reaction microscope. Depending on the CEP of the laser pulses we see a clear asymmetry in the emission direction of the created protons. Contrary to earlier measurements by Kling et al. we observe the highest asymmetry for kinetic energy releases (proton energy) between 0-2 eV. This excludes the electron re-collision mechanism suggested in [1] as dominant excitation channel and requires another explanation.

  17. Transient optical transmission changes induced by pulsed electron radiation in commercial crown silicate glasses

    Science.gov (United States)

    Volchek, A. O.; Lisitsyn, V. M.; Gusarov, A. I.; Yakovlev, V. Yu.; Arbuzov, V. I.

    2003-09-01

    We report on results of time-resolved induced optical absorption measurements in commercial crown silicate glass K8 (similar to Schott BK7 glass) and its radiation-resistant counterpart K108 under 0.25-MeV pulsed electron radiation. The spectra have been obtained in a wavelength range 280-1100 nm on a time interval 10 ns-1 s after the end of a 20-ns pulse. In contrast to behavior of stable defects, the efficiency of non-stationary color centers' generation in the long-wavelength spectrum range is similar for both standard and radiation-resistant glasses. The characteristic time for transmission recovery in the visible range at room temperature was found to be about 100 μs. Based on the Kramers-Krönig relations we have estimated transient refractive index changes. For the same radiation dose such changes can be two orders of magnitude higher than those observed in stationary conditions.

  18. 6 MeV pulsed electron beam induced surface and structural changes in polyimide

    Energy Technology Data Exchange (ETDEWEB)

    Mathakari, Narendra L.; Bhoraskar, Vasant N. [Microtron Accelerator Laboratory, Department of Physics, University of Pune, Ganeshkhind, Pune 411007, Maharashtra (India); Dhole, Sanjay D., E-mail: sanjay@physics.unipune.ernet.i [Microtron Accelerator Laboratory, Department of Physics, University of Pune, Ganeshkhind, Pune 411007, Maharashtra (India)

    2010-04-15

    Thin films of polyimide (PMDA-ODA, Kapton) having 50 mum thickness were irradiated with 6 MeV pulsed electron beam. The bulk and surface properties of pristine and irradiated samples were characterized by several techniques such as stress-strain measurements, Fourier Transform Infrared (FTIR), UV-vis spectroscopy, contact angle, atomic force microscopy (AFM) and profilometry. The tensile strength, percentage elongation and strain energy show an enhancement from pristine value of 73-89 MPa, 10-22% and 4.75-14.2 MJ/m{sup 3} respectively at the maximum fluence of 4 x 10{sup 15} electrons/cm{sup 2}. This signifies that polyimide being an excessively aromatic polymer is crosslinked due to high-energy electron irradiation. In surface properties, the contact angle shows a significant decrease from 59 deg. to 32 deg. indicating enhancement in hydrophilicity. This mainly attributes to surface roughening, which is due to the electron beam induced sputtering. The surface roughening is confirmed in AFM and profilometry measurements. The AFM images clearly show that surface roughness increases after electron irradiation. Moreover, the roughness average (R{sub a}) as measured from surface profilograms is found to increase from 0.06 to 0.1. The FTIR and UV-vis spectra do not show noticeable changes as regards to scissioning of bonds and the oxidation. This work leads to a definite conclusion that 6 MeV pulsed electron beam can be used to bring about desired changes in surface as well as bulk properties of polyimide, which is considered to be a high performance space quality polymer.

  19. Attosecond chirp-encoded dynamics of light nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Haessler, S; Boutu, W; Weber, S; Breger, P; Monchicourt, P; Carre, B; Salieres, P [CEA Saclay, IRAMIS, Service des Photons, Atomes et Molecules, 91191 Gif-sur-Yvette (France); Stankiewicz, M [Institute of Physics, Jagiellonian University, ul. Reymonta 4, 30-059 Krakow (Poland); Frasinski, L J [The Blackett Laboratory, Imperial College London, South Kensington Campus, London SW7 2AZ (United Kingdom); Caillat, J; Taieb, R; Maquet, A [UMPC Universite Paris 06, CNRS, UMR 7614, LCPMR, 11 rue Pierre et Marie Curie, 75231 Paris Cedex 05 (France)], E-mail: pascal.salieres@cea.fr

    2009-07-14

    We study the spectral phase of high-order harmonic emission as an observable for probing ultrafast nuclear dynamics after the ionization of a molecule. Using a strong-field approximation theory that includes nuclear dynamics, we relate the harmonic phase to the phase of the overlap integral of the nuclear wavefunctions of the initial neutral molecule and the molecular ion after an attosecond probe delay. We determine experimentally the group delay of the high harmonic emission from D{sub 2} and H{sub 2} molecules, which allows us to verify the relation between harmonic frequency and the attosecond delay. The small difference in the harmonic phase between H{sub 2} and D{sub 2} calculated theoretically is consistent with our experimental results.

  20. Nonlinear delayed symmetry breaking in a solid excited by hard x-ray free electron laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Ferrer, A., E-mail: aferrer@phys.ethz.ch [Institute for Quantum Electronics, ETH Zurich, CH-8093 Zurich (Switzerland); Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland); Johnson, J. A., E-mail: jjohnson@chem.byu.edu; Mariager, S. O.; Grübel, S.; Staub, U. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland); Huber, T.; Trant, M.; Johnson, S. L., E-mail: johnson@phys.ethz.ch [Institute for Quantum Electronics, ETH Zurich, CH-8093 Zurich (Switzerland); Zhu, D.; Chollet, M.; Robinson, J.; Lemke, H. T. [LCLS, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Ingold, G.; Beaud, P. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland); SwissFEL, Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland); Milne, C. [SwissFEL, Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland)

    2015-04-13

    We have studied the ultrafast changes of electronic states in bulk ZnO upon intense hard x-ray excitation from a free electron laser. By monitoring the transient anisotropy induced in an optical probe beam, we observe a delayed breaking of the initial c-plane symmetry of the crystal that lasts for several picoseconds. Interaction with the intense x-ray pulses modifies the electronic state filling in a manner inconsistent with a simple increase in electronic temperature. These results may indicate a way to use intense ultrashort x-ray pulses to investigate high-energy carrier dynamics and to control certain properties of solid-state materials.

  1. Optical gating and streaking of free electrons with sub-optical cycle precision

    Science.gov (United States)

    Kozák, M.; McNeur, J.; Leedle, K. J.; Deng, H.; Schönenberger, N.; Ruehl, A.; Hartl, I.; Harris, J. S.; Byer, R. L.; Hommelhoff, P.

    2017-01-01

    The temporal resolution of ultrafast electron diffraction and microscopy experiments is currently limited by the available experimental techniques for the generation and characterization of electron bunches with single femtosecond or attosecond durations. Here, we present proof of principle experiments of an optical gating concept for free electrons via direct time-domain visualization of the sub-optical cycle energy and transverse momentum structure imprinted on the electron beam. We demonstrate a temporal resolution of 1.2±0.3 fs. The scheme is based on the synchronous interaction between electrons and the near-field mode of a dielectric nano-grating excited by a femtosecond laser pulse with an optical period duration of 6.5 fs. The sub-optical cycle resolution demonstrated here is promising for use in laser-driven streak cameras for attosecond temporal characterization of bunched particle beams as well as time-resolved experiments with free-electron beams. PMID:28120930

  2. Small-scale electron density and magnetic-field structures in the wake of an ultraintense laser pulse.

    Science.gov (United States)

    Liseikina, T V; Califano, F; Vshivkov, V A; Pegoraro, F; Bulanov, S V

    1999-11-01

    We investigate the interaction of a high intensity ultrashort laser pulse with an underdense collisionless plasma in the regime where the Langmuir wake wave excited behind the laser pulse is loaded by fast particle beams, formed during the wake wave breaking. The beam loading causes the deterioration of the central part of the wake wave near the pulse axis, and the formation of bunches of sharply focalized ultrarelativistic electrons. The bunches of electrons generate a fast propagating magnetic field, which we interpret in terms of the magnetic component of the Lienard-Wiechert potential of a moving electric charge.

  3. Generation of High-Power High-Intensity Short X-Ray Free-Electron-Laser Pulses.

    Science.gov (United States)

    Guetg, Marc W; Lutman, Alberto A; Ding, Yuantao; Maxwell, Timothy J; Decker, Franz-Josef; Bergmann, Uwe; Huang, Zhirong

    2018-01-05

    X-ray free-electron lasers combine a high pulse power, short pulse length, narrow bandwidth, and high degree of transverse coherence. Any increase in the photon pulse power, while shortening the pulse length, will further push the frontier on several key x-ray free-electron laser applications including single-molecule imaging and novel nonlinear x-ray methods. This Letter shows experimental results at the Linac Coherent Light Source raising its maximum power to more than 300% of the current limit while reducing the photon pulse length to 10 fs. This was achieved by minimizing residual transverse-longitudinal centroid beam offsets and beam yaw and by correcting the dispersion when operating over 6 kA peak current with a longitudinally shaped beam.

  4. Pulsed electron beam precharger. Final report, September 1, 1989--May 31, 1992

    Energy Technology Data Exchange (ETDEWEB)

    Finney, W.C. [ed.; Shelton, W.N.

    1992-12-31

    This is the fifth in a series of contracts and grants exploring the advanced particulate pollution control technology of electron beam precipitation. The project currently under contract with the Pittsburgh Energy Technology Center, US DOE, addresses the pressing problem of more efficiently controlling the emission of fine, high resistivity fly ash from low sulfur coal-burning power plants. As such, the project is an integral part of the DOE mission to advance technologies which provide for the safe and economically viable utilization of the nation`s large but potentially polluting coal resources. Within the University Coal Research Program of the DOE, the objective of the project is also consistent with the goal of improving the performance of electrostatic precipitators and possibly fabric filters through the use of a first-stage electron beam particle precharger. Reducing the emission of particulate matter from coal fired boilers is in the national interest from a respiratory health standpoint, while improved power efficiency of the removal process serves the goals of lowered energy consumption. In addition, an earlier spinoff of the ongoing program at FSU was the invention of a new technology using pulsed streamer corona for SO{sub 2} and NO{sub x} removal, the pulse energized electron reactor (PEER) process.

  5. Effect of picosecond magnetic pulse on dynamics of electron's subbands in semiconductor bilayer nanowire

    Science.gov (United States)

    Chwiej, T.

    2017-10-01

    We report on possibility of charge current generation in nanowire made of two tunnel coupled one-dimensional electron waveguides by means of single magnetic pulse lasting up to 20 ps. Existence of interlayer tunnel coupling plays a crucial role in the effect described here as it allows for hybridization of the wave functions localized in different layers which can be dynamically modified by applying a time changeable in-plane magnetic field. Results of time-dependent DFT calculations performed for a bilayer nanowire confining many electrons show that the effect of such magnetic hybridization relies on tilting of electrons' energy subbands, to the left or to the right, depending on a sign of time derivative of oscillating magnetic field due to the Faraday law. Consequently, the tilted subbands become a source of charge flow along the wire. Strength of such magneto-induced current oscillations may achieve even 0.6 μA but it depends on duration of magnetic pulse as well as on charge density confined in nanowire which has to be unequally distributed between both transport layers to observe this effect.

  6. Spectral Interferometry with Electron Microscopes

    Science.gov (United States)

    Talebi, Nahid

    2016-09-01

    Interference patterns are not only a defining characteristic of waves, but also have several applications; characterization of coherent processes and holography. Spatial holography with electron waves, has paved the way towards space-resolved characterization of magnetic domains and electrostatic potentials with angstrom spatial resolution. Another impetus in electron microscopy has been introduced by ultrafast electron microscopy which uses pulses of sub-picosecond durations for probing a laser induced excitation of the sample. However, attosecond temporal resolution has not yet been reported, merely due to the statistical distribution of arrival times of electrons at the sample, with respect to the laser time reference. This is however, the very time resolution which will be needed for performing time-frequency analysis. These difficulties are addressed here by proposing a new methodology to improve the synchronization between electron and optical excitations through introducing an efficient electron-driven photon source. We use focused transition radiation of the electron as a pump for the sample. Due to the nature of transition radiation, the process is coherent. This technique allows us to perform spectral interferometry with electron microscopes, with applications in retrieving the phase of electron-induced polarizations and reconstructing dynamics of the induced vector potential.

  7. Properties of Silicon Dioxide Amorphous Nanopowder Produced by Pulsed Electron Beam Evaporation

    Directory of Open Access Journals (Sweden)

    Vladislav G. Il’ves

    2015-01-01

    Full Text Available SiO2 amorphous nanopowder (NP is produced with the specific surface area of 154 m2/g by means of evaporation by a pulsed electron beam aimed at Aerosil 90 pyrogenic amorphous NP (90 m2/g as a target. SiO2 NP nanoparticles showed improved magnetic, thermal, and optical properties in comparison to Aerosil 90 NP. Possible reasons of emergence of d0 ferromagnetism at the room temperature in SiO2 amorphous NP are discussed. Photoluminescent and cathode luminescent properties of the SiO2 NP were investigated.

  8. Role of sublayers in mechanical response of pulsed electron beam irradiated surface layers to contact load

    Science.gov (United States)

    Konovalenko, Igor S.

    2017-12-01

    Here we develop the movable cellular automaton method based a numerical model of surface layers in a NiCr-TiC metal ceramic composite modified by pulsed electron beam irradiation in inert gas plasmas. The model explicitly takes into account the presence of several sublayers differing in structure and mechanical properties. The contribution of each sublayer to the mechanical response of the modified surface to contact loading is studied. It is shown that the maximum strength and fracture toughness are achieved in surface layers containing thin and stiff external sublayers and a more ductile thick internal sublayer.

  9. Extended Pulse-Powered Humidity-Freeze Cycling for Testing Module-Level Power Electronics

    Energy Technology Data Exchange (ETDEWEB)

    Hacke, Peter L [National Renewable Energy Laboratory (NREL), Golden, CO (United States); Rodriguez, Miguel [National Renewable Energy Laboratory (NREL), Golden, CO (United States); Kempe, Michael D [National Renewable Energy Laboratory (NREL), Golden, CO (United States); Repins, Ingrid L [National Renewable Energy Laboratory (NREL), Golden, CO (United States)

    2017-11-28

    An EMI suppression capacitor (polypropylene film type) failed by 'popcorning' due to vapor outgassing in pulse powered humidity-freeze cycles. No shorts or shunts could be detected despite mildly corroded metallization visible in the failed capacitor. Humidity-freeze cycling is optimized to break into moisture barriers. However, further studies will be required on additional module level power electronic (MLPE) devices to optimize the stress testing for condensation to precipitate any weakness to short circuiting and other humidity/bias failure modes.

  10. Formation of Surface Nano- and Textured Austenite Induced by Pulsed Electron Beam Irradiation under Melting Mode

    Directory of Open Access Journals (Sweden)

    K. M. Zhang

    2013-01-01

    Full Text Available We report in this paper an interesting phenomenon associated with low-energy high-current pulsed electron beam (LEHCPEB treatment: surface nanograined and textured austenite formation under the melting treatment mode. The treatment induces superfast heating and melting followed by a rapid solidification and cooling of the material surfaces. As a result, nano-structured surface layers can be achieved quite easily. Examples of nanoaustenite formation with special texture state in the modified surface layer of AISI D2 steel and NiTi alloy will show the potential for surface nanocrystallization of materials with improved properties by LEHCPEB technique.

  11. Beam dynamics analysis in pulse compression using electron beam compact simulator for Heavy Ion Fusion

    Directory of Open Access Journals (Sweden)

    Kikuchi Takashi

    2013-11-01

    Full Text Available In a final stage of an accelerator system for heavy ion inertial fusion (HIF, pulse shaping and beam current increase by bunch compression are required for effective pellet implosion. A compact simulator with an electron beam was constructed to understand the beam dynamics. In this study, we investigate theoretically and numerically the beam dynamics for the extreme bunch compression in the final stage of HIF accelerator complex. The theoretical and numerical results implied that the compact experimental device simulates the beam dynamics around the stagnation point for initial low temperature condition.

  12. Investigation of industrial-scale carbon dioxide reduction using pulsed electron beams

    Energy Technology Data Exchange (ETDEWEB)

    Petrov, G. M.; Apruzese, J. P.; Petrova, Tz. B.; Wolford, M. F. [Plasma Physics Division, Naval Research Laboratory, 4555 Overlook Ave. SW, Washington, DC 20375-5346 (United States)

    2016-03-14

    Carbon dioxide is the most important greenhouse gas contributing to global warming. To help mitigate increasing CO{sub 2} concentrations, we investigate a method of carbon dioxide reduction using high-power electron beams, which can be used on an industrial scale. A series of experiments are conducted in which the reduction of CO{sub 2} is measured for different gas compositions and power deposition rates. An electron beam deposition model is applied to compute reduction rates of CO{sub 2} and energy cost for breaking a CO{sub 2} molecule in flue gas and pure carbon dioxide at atmospheric pressure. For flue gas consisting of 82% N{sub 2}, 6% O{sub 2}, and 12% CO{sub 2}, the calculated energy cost is 85 eV per molecule. In order to dissociate 50% of the CO{sub 2} molecules, beam energy density deposition on the order of 20 J/cm{sup 3} is required. Electron beam irradiation of 12.6 liter gas volume containing 90% CO{sub 2} and 10% CH{sub 4} at beam energy density deposition of 4.2 J/cm{sup 3}, accumulated over 43 shots in a 20 min interval, reduced the CO{sub 2} concentration to 78%. Analogous experiments with a gas mixture containing 11.5% CO{sub 2}, 11.5% CH{sub 4}, and balance of Ar, reduced the CO{sub 2} concentration to below 11% with energy deposition 0.71 J/cm{sup 3}, accumulated over 10 shots in a 5 min interval. The experimental data and the theoretical predictions of CO{sub 2} reduction using pulsed electron beams are in agreement within the experimental error. Other techniques to enhance the removal of CO{sub 2} with pulsed electron beams are also explored, yielding new possible avenues of research.

  13. Science at the Time-scale of the Electron

    Science.gov (United States)

    Murnane, Margaret

    2010-03-01

    Replace this text with your abstract Ever since the invention of the laser 50 years ago and its application in nonlinear optics, scientists have been striving to extend coherent laser beams into the x-ray region of the spectrum. Very recently however, the prospects for tabletop coherent sources, with attosecond pulse durations, at very short wavelengths even in the hard x-ray region of the spectrum at wavelengths new ability to manipulate electrons on the fastest, attosecond, time-scales of our natural world. My talk will discuss new experimental data that demonstrates high harmonic generation of laser-like, fully coherent, 10 attosecond duration, soft x-ray beams at photon energies around 0.5keV. Several applications will also be discussed, including making a movie of how electron orbitals in a molecule change shape as a molecule breaks apart, following how fast a magnetic material can flip orientation, understanding how fast heat flows in a nanocircuit, or building a microscope without lenses. [4pt] [1] T. Popmintchev et al., ``Phase matched upconversion of coherent ultrafast laser light into the soft and hard x-ray regions of the spectrum'', PNAS 106, 10516 (2009). [0pt] [2] C. LaOVorakiat et al., ``Ultrafast Soft X-Ray Magneto-Optics at the M-edge Using a Tabletop High-Harmonic Source'', Physical Review Letters 103, 257402 (2009). [0pt] [3] M. Siemens et al. ``Measurement of quasi-ballistic heat transport across nanoscale interfaces using ultrafast coherent soft x-ray beams'', Nature Materials 9, 26 (2010). [0pt] [4] K. Raines et al., ``Three-dimensional structure determination from a single view,'' Nature 463, 214 (2010). [0pt] [5] W. Li et al., ``Time-resolved Probing of Dynamics in Polyatomic Molecules using High Harmonic Generation'', Science 322, 1207 (2008).

  14. New injection scheme using a pulsed quadrupole magnet in electron storage rings

    Directory of Open Access Journals (Sweden)

    Kentaro Harada

    2007-12-01

    Full Text Available We demonstrated a new injection scheme using a single pulsed quadrupole magnet (PQM with no pulsed local bump at the Photon Factory Advanced Ring (PF-AR in High Energy Accelerator Research Organization (KEK. The scheme employs the basic property of a quadrupole magnet, that the field at the center is zero, and nonzero elsewhere. The amplitude of coherent betatron oscillation of the injected beam is effectively reduced by the PQM; then, the injected beam is captured into the ring without largely affecting the already stored beam. In order to investigate the performance of the scheme with a real beam, we built the PQM providing a higher field gradient over 3  T/m and a shorter pulse width of 2.4  μs, which is twice the revolution period of the PF-AR. After the field measurements confirmed the PQM specifications, we installed it into the ring. Then, we conducted the experiment using a real beam and consequently succeeded in storing the beam current of more than 60 mA at the PF-AR. This is the first successful beam injection using a single PQM in electron storage rings.

  15. Longitudinal injection scheme using short pulse kicker for small aperture electron storage rings

    Directory of Open Access Journals (Sweden)

    M. Aiba

    2015-02-01

    Full Text Available Future light sources aim at achieving a diffraction limited photon beam both in the horizontal and vertical planes. High gradient quadrupoles and strong chromaticity correction sextupoles in a corresponding ultra-low emittance ring may restrict the physical and dynamic aperture of the storage ring such that off-axis injection and accumulation may become impossible. We propose a longitudinal injection scheme, i.e., injecting an electron bunch onto the closed orbit with a time offset with respect to the circulating bunches. The temporal separation enables a pulsed dipole kicker to situate the injected bunch transversely on-axis without disturbing the circulating bunches if the pulse length is shorter than the bunch spacing. The injected bunch is finally merged to a circulating bunch through synchrotron radiation damping. We present the scheme in detail and its application to the lattice of the MAX IV 3 GeV storage ring. The requirements and feasibility of the pulsed dipole kicker are also discussed.

  16. Relativistic electron beams driven by kHz single-cycle light pulses

    CERN Document Server

    Guénot, D; Vernier, A; Beaurepaire, B; Böhle, F; Bocoum, M; Lozano, M; Jullien, A; Lopez-Martens, R; Lifschitz, A; Faure, J

    2016-01-01

    Laser-plasma acceleration is an emerging technique for accelerating electrons to high energies over very short distances. The accelerated electron bunches have femtosecond duration, making them particularly relevant for applications such as ultrafast imaging or femtosecond X-ray generation. Current laser-plasma accelerators are typically driven by Joule-class laser systems that have two main drawbacks: their relatively large scale and their low repetition-rate, with a few shots per second at best. The accelerated electron beams have energies ranging from 100 MeV to multi-GeV, however a MeV electron source would be more suited to many societal and scientific applications. Here, we demonstrate a compact and reliable laser-plasma accelerator producing high-quality few-MeV electron beams at kilohertz repetition rate. This breakthrough was made possible by using near-single-cycle light pulses, which lowered the required laser energy for driving the accelerator by three orders of magnitude, thus enabling high repet...

  17. Momentum mapping of continuum electron wave packet interference

    CERN Document Server

    Yang, Weifeng; Lin, Cheng; Xu, Jingwen; Sheng, Zhihao; Song, Xiaohong; Hu, Shilin; Chen, Jing

    2016-01-01

    We analyze the two-dimensional photoelectrons momentum distribution of Ar atom ionized by midinfrared laser pulses and mainly concentrate on the energy range below 2Up. By using a generalized quantum trajectory Monte Carlo (GQTMC) simulation and comparing with the numerical solution of time-dependent Schrodinger equation (TDSE), we show that in the deep tunneling regime, the rescattered electron trajectories plays unimportant role and the interplay between the intracycle and inter-cycle results in a ring-like interference pattern. The ring-like interference pattern will mask the holographic interference structure in the low longitudinal momentum region. When the nonadiabatic tunneling contributes significantly to ionization, i.e., the Keldysh parameter 1, the contribution of the rescattered electron trajectories become large, thus holographic interference pattern can be clearly observed. Our results help paving the way for gaining physical insight into ultrafast electron dynamic process with attosecond tempor...

  18. Attosecond-recollision-controlled selective fragmentation of polyatomic molecules.

    Science.gov (United States)

    Xie, Xinhua; Doblhoff-Dier, Katharina; Roither, Stefan; Schöffler, Markus S; Kartashov, Daniil; Xu, Huailiang; Rathje, Tim; Paulus, Gerhard G; Baltuška, Andrius; Gräfe, Stefanie; Kitzler, Markus

    2012-12-14

    Control over various fragmentation reactions of a series of polyatomic molecules (acetylene, ethylene, 1,3-butadiene) by the optical waveform of intense few-cycle laser pulses is demonstrated experimentally. We show both experimentally and theoretically that the responsible mechanism is inelastic ionization from inner-valence molecular orbitals by recolliding electron wave packets, whose recollision energy in few-cycle ionizing laser pulses strongly depends on the optical waveform. Our work demonstrates an efficient and selective way of predetermining fragmentation and isomerization reactions in polyatomic molecules on subfemtosecond time scales.

  19. Surface Modification of Light Alloys by Low-Energy High-Current Pulsed Electron Beam

    Directory of Open Access Journals (Sweden)

    X. D. Zhang

    2012-01-01

    Full Text Available This paper reviews results obtained by the research groups developing the low-energy high-current pulsed electron beam (LEHCPEB in Dalian (China and Metz (France on the surface treatment of light alloys. The pulsed electron irradiation induces an ultra-fast thermal cycle at the surface combined with the formation of thermal stress and shock waves. As illustrated for Mg alloys and Ti, this results in deep subsurface hardening (over several 100 μm which improves the wear resistance. The analysis of the top surface melted surface of light alloys also often witnesses evaporation and condensation of chemical species. This phenomenon can significantly modify the melt chemistry and was also suggested to lead to the development of specific solidification textures in the rapidly solidified layer. The potential use of the LEHCPEB technique for producing thermomechanical treatments under the so-called heating mode and, thus, modify the surface crystallographic texture, and enhance solid-state diffusion is also demonstrated in the case of the FeAl intermetallic compound.

  20. High-throughput rear-surface drilling of microchannels in glass based on electron dynamics control using femtosecond pulse trains.

    Science.gov (United States)

    Jiang, Lan; Liu, Pengjun; Yan, Xueliang; Leng, Ni; Xu, Chuancai; Xiao, Hai; Lu, Yongfeng

    2012-07-15

    This study proposes a rear-surface ablation enhancement approach to fabricate high-aspect-ratio microchannels by temporally shaping femtosecond laser pulse trains. In the case study of K9 glass, enhancements of up to a 56 times higher material removal rate and a three times greater maximum drilling depth are obtained by the proposed method, as compared with conventional femtosecond laser drilling at the same processing parameters. The improvements are due to the changes of photon-electron interactions by shaping femtosecond pulse train, which can effectively adjust the photon absorption and localized transient material properties by changing electron dynamics such as free electron densities.

  1. Correlation-driven charge migration following double ionization and attosecond transient absorption spectroscopy

    Science.gov (United States)

    Hollstein, Maximilian; Santra, Robin; Pfannkuche, Daniela

    2017-05-01

    We theoretically investigate charge migration following prompt double ionization. Thereby, we extend the concept of correlation-driven charge migration, which was introduced by Cederbaum and coworkers for single ionization [Chem. Phys. Lett. 307, 205 (1999), 10.1016/S0009-2614(99)00508-4], to doubly ionized molecules. This allows us to demonstrate that compared to singly ionized molecules, in multiply ionized molecules, electron dynamics originating from electronic relaxation and correlation are particularly prominent. In addition, we also discuss how these correlation-driven electron dynamics might be evidenced and traced experimentally using attosecond transient absorption spectroscopy. For this purpose, we determine the time-resolved absorption cross section and find that the correlated electron dynamics discussed are reflected in it with exceptionally great detail. Strikingly, we find that features in the cross section can be traced back to electron hole populations and time-dependent partial charges and hence, can be interpreted with surprising ease. By taking advantage of element-specific core-to-valence transitions even atomic spatial resolution can be achieved. Thus, with the theoretical considerations presented, not only do we predict particularly diverse and correlated electron dynamics in molecules to follow prompt multiple ionization but we also identify a promising route towards their experimental investigation.

  2. Picosecond imaging of inertial confinement fusion plasmas using electron pulse-dilation

    Science.gov (United States)

    Hilsabeck, T. J.; Nagel, S. R.; Hares, J. D.; Kilkenny, J. D.; Bell, P. M.; Bradley, D. K.; Dymoke-Bradshaw, A. K. L.; Piston, K.; Chung, T. M.

    2017-02-01

    Laser driven inertial confinement fusion (ICF) plasmas typically have burn durations on the order of 100 ps. Time resolved imaging of the x-ray self emission during the hot spot formation is an important diagnostic tool which gives information on implosion symmetry, transient features and stagnation time. Traditional x-ray gated imagers for ICF use microchannel plate detectors to obtain gate widths of 40-100 ps. The development of electron pulse-dilation imaging has enabled a 10X improvement in temporal resolution over legacy instruments. In this technique, the incoming x-ray image is converted to electrons at a photocathode. The electrons are accelerated with a time-varying potential that leads to temporal expansion as the electron signal transits the tube. This expanded signal is recorded with a gated detector and the effective temporal resolution of the composite system can be as low as several picoseconds. An instrument based on this principle, known as the Dilation X-ray Imager (DIXI) has been constructed and fielded at the National Ignition Facility. Design features and experimental results from DIXI will be presented.

  3. Parametric generation of energetic short mid-infrared pulses for dielectric laser acceleration

    Science.gov (United States)

    Wandel, S.; Xu, G.; Yin, Y.; Jovanovic, I.

    2014-12-01

    Laser-driven high-gradient electron acceleration in dielectric photonic structures is an enabling technology for compact and robust sources of tunable monochromatic x-rays. Such advanced x-ray sources are sought in medical imaging, security, industrial, and scientific applications. The use of long-wavelength pulses can mitigate the problem of laser-induced breakdown in dielectric structures at high optical intensities, relax the structure fabrication requirements, and allow greater pulse energy to be injected into the structure. We report on the design and construction of a simple and robust, short-pulse parametric source operating at a center wavelength 5 μm, to be used as a pump for a dielectric photonic structure for laser-driven acceleration. The source is based on a two-stage parametric downconversion design, consisting of a β-BaB2O4-based 2.05 μm optical parametric amplifier (OPA) and a ZnGeP2-based 5 μm OPA. The 2.05 μm OPA is presently pumped by a standard Ti:sapphire chirped-pulse amplified laser, which will be replaced with direct laser pumping at wavelengths \\gt 2 μ m in the future. The design and performance of the constructed short-pulse mid-infrared source are described. The demonstrated architecture is also of interest for use in other applications, such as high harmonic generation and attosecond pulse production.

  4. Electron-ion relaxation time dependent signal enhancement in ultrafast double-pulse laser-induced breakdown spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Harilal, S. S.; Diwakar, P. K.; Hassanein, A. [Center for Materials Under Extreme Environment, School of Nuclear Engineering, Purdue University, West Lafayette, Indiana 47907 (United States)

    2013-07-22

    We investigated the emission properties of collinear double-pulse compared to single-pulse ultrafast laser induced breakdown spectroscopy. Our results showed that the significant signal enhancement noticed in the double pulse scheme is strongly correlated to the characteristic electron-ion relaxation time and hence to the inter-pulse delays. Spectroscopic excitation temperature analysis showed that the improvement in signal enhancement is caused by the delayed pulse efficient reheating of the pre-plume. The signal enhancement is also found to be related to the upper excitation energy of the selected lines, i.e., more enhancement noticed for lines originating from higher excitation energy levels, indicating reheating is the major mechanism behind the signal improvement.

  5. Electron-ion relaxation time dependent signal enhancement in ultrafast double-pulse laser-induced breakdown spectroscopy

    Science.gov (United States)

    Harilal, S. S.; Diwakar, P. K.; Hassanein, A.

    2013-07-01

    We investigated the emission properties of collinear double-pulse compared to single-pulse ultrafast laser induced breakdown spectroscopy. Our results showed that the significant signal enhancement noticed in the double pulse scheme is strongly correlated to the characteristic electron-ion relaxation time and hence to the inter-pulse delays. Spectroscopic excitation temperature analysis showed that the improvement in signal enhancement is caused by the delayed pulse efficient reheating of the pre-plume. The signal enhancement is also found to be related to the upper excitation energy of the selected lines, i.e., more enhancement noticed for lines originating from higher excitation energy levels, indicating reheating is the major mechanism behind the signal improvement.

  6. Single-Molecule Imaging with X-Ray Free-Electron Lasers: Dream or Reality?

    KAUST Repository

    Fratalocchi, Andrea

    2011-03-09

    X-ray free-electron lasers (XFEL) are revolutionary photon sources, whose ultrashort, brilliant pulses are expected to allow single-molecule diffraction experiments providing structural information on the atomic length scale of nonperiodic objects. This ultimate goal, however, is currently hampered by several challenging questions basically concerning sample damage, Coulomb explosion, and the role of nonlinearity. By employing an original ab initio approach, we address these issues showing that XFEL-based single-molecule imaging will be only possible with a few-hundred long attosecond pulses, due to significant radiation damage and the formation of preferred multisoliton clusters which reshape the overall electronic density of the molecular system at the femtosecond scale.

  7. Attosecond-correlated dynamics of two electrons in argon

    Indian Academy of Sciences (India)

    2014-01-11

    Planck-Institut für Quantenoptik, 85748 Garching, Germany. 5Physikalisch Technische Bundesanstalt, 38116 Braunschweig, Germany. ∗. Corresponding author. E-mail: vsharma@iith.ac.in. DOI: 10.1007/s12043-013-0645-x; ...

  8. Pulsed electron beam deposition of transparent conducting Al-doped ZnO films

    Energy Technology Data Exchange (ETDEWEB)

    Quang, Pham Hong, E-mail: phquang2711@yahoo.com [Hanoi University of Science, Vietnam National University, Hanoi, 334 Nguyen Trai, Thanh Xuan, Hanoi (Viet Nam); Sang, Ngo Dinh [National University of Civil Engineering, 55 Giai Phong Street, Hai Ba Trung, Hanoi (Viet Nam); Ngoc, Do Quang [Hanoi University of Science, Vietnam National University, Hanoi, 334 Nguyen Trai, Thanh Xuan, Hanoi (Viet Nam)

    2012-08-31

    Good quality transparent conducting Al-doped ZnO films were deposited on quartz substrates from a high purity target using pulsed electron deposition (PED). Two series of films were made, one deposited at room temperature but at four pressures, viz., 0.7, 1.3, 2.0 and 2.7 Pa of oxygen and one deposited at 1.3 Pa oxygen pressure but at the substrate temperature ranged from room temperature to 600 Degree-Sign C. In order to evaluate the effect of substrate temperature and oxygen pressure on the properties of obtained films, various characterization techniques were employed including X-ray diffraction, stylus profiler, scanning electron microscope, optical spectrophotometer and electrical resistivity. For the first series films, the optimal oxygen pressure of 1.3 Pa was found to bring about the appropriate energetic deposition atoms which results in the best crystallinity. For the second series films, the lowest resistivity was obtained in the film grown at 400 Degree-Sign C. An attempt was made to reduce the resistivity by lowering the oxygen pressure to 0.5 Pa which was the lower limit of working pressure of the PED system. The obtained results indicate that PED is a suitable technique for growing transparent conducting ZnO films. - Highlights: Black-Right-Pointing-Pointer Transparent conducting Al-doped ZnO films grown by pulsed electron deposition (PED). Black-Right-Pointing-Pointer The film properties were found to depend strongly on the deposition conditions. Black-Right-Pointing-Pointer The best film was grown at the oxygen pressure of 0.5 Pa and at 400 Degree-Sign C. Black-Right-Pointing-Pointer PED is found to be a suitable technique for growing transparent conducting ZnO films.

  9. Development of a 4.5 K Pulse Tube Cryocooler for Superconducting Electronics

    Science.gov (United States)

    Nast, Ted; Olson, Jeff; Champagne, Patrick; Mix, Jack; Evtimov, Bobby; Roth, Eric; Collaco, Andre

    2008-03-01

    Lockheed Martin's (LM) Advanced Technology Center (ATC) has developed a four stage pulse tube cryocooler (stirling-type pulse tube system) to provide cooling at 4.5 K for superconducting digital electronics communications programs. These programs utilize superconducting niobium integrated circuits [1, 2]. A prior ATC 4 stage unit has provided cooling to 3.8 K. [3] The relatively high cooling loads for the present program led us to a new design which improves the 4.5 K power efficiency over prior systems. This design includes a unique pulse tube approach using both He-3 and He-4 working gas in two compression spaces. The compressor utilizes our standard moving magnet linear motor, clearance seal and flexure bearing system. The system is compact, lightweight and reliable and utilizes our aerospace cooler technology to provide unlimited lifetime. The unit is a proof of concept, but the construction is at an engineering model level. Follow on activities for improvements of performance and more compact packaging and future production for ground based communication systems is anticipated. This paper presents the experimental results at various cooling conditions. Primary results are shown for HYPRES cooling requirements and data is also included at lower cooling loads that may be required for future space missions. The system provides a maximum of 42 mW @ 4.5 K and a no load temperature of 3 K. The majority of this work was subcontracted by HYPRES and funded by the Army and Navy. A small part of this effort to obtain data at lower cooling loads (1-10 mW @ 4.5 K) was funded by LM internal funds.

  10. Microstructure Modifications and Associated Corrosion Improvements in GH4169 Superalloy Treated by High Current Pulsed Electron Beam

    Directory of Open Access Journals (Sweden)

    Yichang Su

    2015-01-01

    Full Text Available The surface of the nickel-based superalloy GH4169 was subjected to high-current pulsed electron beam (HCPEB treatment. The microstructural morphologies of the material were analysed by means of optical microscope (OP, scanning electron microscope (SEM, and transmission electron microscope (TEM. The results reveal that the irradiated surface was remelted and many craters were formed. The density of craters decreased with the increment of HCPEB pulses. After 20-pulsed HCPEB irradiation, nanostructures were formed in the melted region of the surface. Furthermore, slipping bands and high density of dislocations were also formed due to the severe plastic deformation. The selective purification effect, homogenized composition, nanostructures, and dislocation slips introduced by HCPEB irradiation bring a significant improvement of corrosion resistance of GH4169 superalloy.

  11. Development of experimental techniques for the characterization of ultrashort photon pulses of extreme ultraviolet free-electron lasers

    Science.gov (United States)

    Düsterer, S.; Rehders, M.; Al-Shemmary, A.; Behrens, C.; Brenner, G.; Brovko, O.; DellAngela, M.; Drescher, M.; Faatz, B.; Feldhaus, J.; Frühling, U.; Gerasimova, N.; Gerken, N.; Gerth, C.; Golz, T.; Grebentsov, A.; Hass, E.; Honkavaara, K.; Kocharian, V.; Kurka, M.; Limberg, Th.; Mitzner, R.; Moshammer, R.; Plönjes, E.; Richter, M.; Rönsch-Schulenburg, J.; Rudenko, A.; Schlarb, H.; Schmidt, B.; Senftleben, A.; Schneidmiller, E. A.; Siemer, B.; Sorgenfrei, F.; Sorokin, A. A.; Stojanovic, N.; Tiedtke, K.; Treusch, R.; Vogt, M.; Wieland, M.; Wurth, W.; Wesch, S.; Yan, M.; Yurkov, M. V.; Zacharias, H.; Schreiber, S.

    2014-12-01

    One of the most challenging tasks for extreme ultraviolet, soft and hard x-ray free-electron laser photon diagnostics is the precise determination of the photon pulse duration, which is typically in the sub 100 fs range. Nine different methods, able to determine such ultrashort photon pulse durations, were compared experimentally at FLASH, the self-amplified spontaneous emission free-electron laser at DESY in Hamburg, in order to identify advantages and disadvantages of different methods. Radiation pulses at a wavelength of 13.5 and 24.0 nm together with the corresponding electron bunch duration were measured by indirect methods like analyzing spectral correlations, statistical fluctuations, and energy modulations of the electron bunch and also by direct methods like autocorrelation techniques, terahertz streaking, or reflectivity changes of solid state samples. In this paper, we present a comprehensive overview of the various techniques and a comparison of the individual experimental results. The information gained is of utmost importance for the future development of reliable pulse duration monitors indispensable for successful experiments with ultrashort extreme ultraviolet pulses.

  12. Development of experimental techniques for the characterization of ultrashort photon pulses of extreme ultraviolet free-electron lasers

    Directory of Open Access Journals (Sweden)

    S. Düsterer

    2014-12-01

    Full Text Available One of the most challenging tasks for extreme ultraviolet, soft and hard x-ray free-electron laser photon diagnostics is the precise determination of the photon pulse duration, which is typically in the sub 100 fs range. Nine different methods, able to determine such ultrashort photon pulse durations, were compared experimentally at FLASH, the self-amplified spontaneous emission free-electron laser at DESY in Hamburg, in order to identify advantages and disadvantages of different methods. Radiation pulses at a wavelength of 13.5 and 24.0 nm together with the corresponding electron bunch duration were measured by indirect methods like analyzing spectral correlations, statistical fluctuations, and energy modulations of the electron bunch and also by direct methods like autocorrelation techniques, terahertz streaking, or reflectivity changes of solid state samples. In this paper, we present a comprehensive overview of the various techniques and a comparison of the individual experimental results. The information gained is of utmost importance for the future development of reliable pulse duration monitors indispensable for successful experiments with ultrashort extreme ultraviolet pulses.

  13. Surface Nanostructure Formations in an AISI 316L Stainless Steel Induced by Pulsed Electron Beam Treatment

    Directory of Open Access Journals (Sweden)

    Yang Cai

    2015-01-01

    Full Text Available High current pulsed electron beam (HCPEB is an efficient technique for surface modifications of metallic materials. In the present work, the formations of surface nanostructures in an AISI 316L stainless steel induced by direct HCPEB treatment and HCPEB alloying have been investigated. After HCPEB Ti alloying, the sample surface contained a mixture of the ferrite and austenite phases with an average grain size of about 90 nm, because the addition of Ti favors the formation of ferrite. In contrast, electron backscattered diffraction (EBSD analyses revealed no structural refinement on the direct HCPEB treated sample. However, transmission electron microscope (TEM observations showed that fine cells having an average size of 150 nm without misorientations, as well as nanosized carbide particles, were formed in the surface layer after the direct HCPEB treatment. The formation of nanostructures in the 316L stainless steel is therefore attributed to the rapid solidification and the generation of different phases other than the steel substrate in the melted layer.

  14. Study on Nanostructures Induced by High-Current Pulsed Electron Beam

    Directory of Open Access Journals (Sweden)

    Bo Gao

    2012-01-01

    Full Text Available Four techniques using high-current pulsed electron beam (HCPEB were proposed to obtain surface nanostructure of metal and alloys. The first method involves the distribution of several fine Mg nanoparticles on the top surface of treated samples by evaporation of pure Mg with low boiling point. The second technique uses superfast heating, melting, and cooling induced by HCPEB irradiation to refine the primary phase or the second phase in alloys to nanosized uniform distributed phases in the matrix, such as the quasicrystal phase Mg30Zn60Y10 in the quasicrystal alloy Mg67Zn30Y3. The third technique involves the refinement of eutectic silicon phase in hypereutectic Al-15Si alloys to fine particles with the size of several nanometers through solid solution and precipitation refinement. Finally, in the deformation zone induced by HCPEB irradiation, the grain size can be refined to several hundred nanometers, such as the grain size of the hypereutectic Al-15Si alloys in the deformation zone, which can reach ~400 nm after HCPEB treatment for 25 pulses. Therefore, HCPEB technology is an efficient way to obtain surface nanostructure.

  15. Digital pulse processing and optimization of the front-end electronics for nuclear instrumentation.

    Science.gov (United States)

    Bobin, C; Bouchard, J; Thiam, C; Ménesguen, Y

    2014-05-01

    This article describes an algorithm developed for the digital processing of signals provided by a high-efficiency well-type NaI(Tl) detector used to apply the 4πγ technique. In order to achieve a low-energy threshold, a new front-end electronics has been specifically designed to optimize the coupling to an analog-to-digital converter (14 bit, 125 MHz) connected to a digital development kit produced by Altera(®). The digital pulse processing is based on an IIR (Infinite Impulse Response) approximation of the Gaussian filter (and its derivatives) that can be applied to the real-time processing of digitized signals. Based on measurements obtained with the photon emissions generated by an (241)Am source, the energy threshold is estimated to be equal to ~2 keV corresponding to the physical threshold of the NaI(Tl) detector. An algorithm developed for a Silicon Drift Detector used for low-energy x-ray spectrometry is also described. In that case, the digital pulse processing is specifically designed for signals provided by a reset-type preamplifier ((55)Fe source). © 2013 Published by Elsevier Ltd.

  16. Electroluminescence pulse shape and electron diffusion in liquid argon measured in a dual-phase TPC

    Energy Technology Data Exchange (ETDEWEB)

    Agnes, P.; et al.

    2018-02-05

    We report the measurement of the longitudinal diffusion constant in liquid argon with the DarkSide-50 dual-phase time projection chamber. The measurement is performed at drift electric fields of 100 V/cm, 150 V/cm, and 200 V/cm using high statistics $^{39}$Ar decays from atmospheric argon. We derive an expression to describe the pulse shape of the electroluminescence signal (S2) in dual-phase TPCs. The derived S2 pulse shape is fit to events from the uppermost portion of the TPC in order to characterize the radial dependence of the signal. The results are provided as inputs to the measurement of the longitudinal diffusion constant DL, which we find to be (4.12 $\\pm$ 0.04) cm$^2$/s for a selection of 140keV electron recoil events in 200V/cm drift field and 2.8kV/cm extraction field. To study the systematics of our measurement we examine datasets of varying event energy, field strength, and detector volume yielding a weighted average value for the diffusion constant of (4.09 $\\pm$ 0.09) cm$^2$ /s. The measured longitudinal diffusion constant is observed to have an energy dependence, and within the studied energy range the result is systematically lower than other results in the literature.

  17. Ghost stochastic resonance with distributed inputs in pulse-coupled electronic neurons

    Science.gov (United States)

    Lopera, Abel; Buldú, Javier M.; Torrent, M. C.; Chialvo, Dante R.; García-Ojalvo, Jordi

    2006-02-01

    We study experimentally the phenomenon of ghost stochastic resonance in pulse-coupled excitable systems, for input signals distributed among different elements. Specifically, two excitable electronic circuits are driven by different sinusoidal signals that produce periodic spikes at distinct frequencies. Their outputs are sent to a third circuit that processes these spiking signals and is additionally perturbed by noise. When the input signals are harmonics of a certain fundamental (that is not present in the inputs) the processing circuit exhibits, for an optimal amount of noise, a resonant response at the frequency of the missing fundamental (ghost frequency). In contrast with the standard case in which the signals being directly integrated are sinusoidal, this behavior relies here on a coincidence-detection mechanism. When the input signals are homogeneously shifted in frequency, the processing circuit responds with pulse packages composed of spikes at a frequency that depends linearly on the frequency shift. Expressions for the dependence of the package period and duration on the frequency shift and spike width, respectively, are obtained. These results provide an experimental verification of a recently proposed mechanism of binaural pitch perception.

  18. Time-resolved mapping of correlated electron emission from helium atom in an intense laser pulse

    Energy Technology Data Exchange (ETDEWEB)

    Ruiz, C; Becker, A [Max-Planck-Institut fuer Physik of Komplexer Systeme, Noethnitzer Str. 38, D-01187 Dresden (Germany)], E-mail: abecker@pks.mpg.de

    2008-02-15

    We apply and analyze the concept of mapping ionization time on to the final momentum distribution to the correlated electron dynamics in the nonsequential double ionization of helium in a strong laser pulse ({lambda}=800 nm) and show how the mapping provides insight into the double ionization dynamics. To this end, we study, by means of numerical integration of the time-dependent Schroedinger equation of a fully correlated model atom, the temporal evolution of the center-of-mass momentum in a short laser pulse. Our results show that in the high intensity regime (I{sub 0}=1.15x10{sup 15} W cm{sup -2}), the mapping is in good agreement with a classical model including binary and recoil rescattering mechanisms. In the medium intensity regime (I{sub 0}=5x10{sup 14} W cm{sup -2}), we identify additional contributions from the recollision-induced excitation of the ion followed by subsequent field ionization (RESI)

  19. Time-resolved mapping of correlated electron emission from helium atom in an intense laser pulse

    Energy Technology Data Exchange (ETDEWEB)

    Ruiz Mendez, Camilo [Max-Planck-Institut fuer Physik Komplexer Systeme, Dresden (Germany)

    2008-07-01

    We apply and analyze the concept of mapping ionization time onto the final momentum distribution to the correlated electron dynamics in the non-sequential double ionization of Helium in a strong laser pulse ({lambda}=800 nm) and show how the mapping provides insight into the double ionization dynamics. To this end, we study by means of numerical integration of the time dependent Schroedinger equation of a fully correlated model atom the temporal evolution of the center-of-mass momentum in a short laser pulse. Our results show that in the high intensity regime (I{sub 0}=1.15 x 10{sup 15} W/cm{sup 2}) the mapping is in good agreement with a classical model including binary and recoil rescattering mechanisms. In the medium intensity regime (I{sub 0}=5 x 10{sup 14} W/cm{sup 2}) we identify additional contributions from the recollision-induced excitation of the ion followed by subsequent field ionization (RESI).

  20. X-ray framing camera for pulsed, high current, electron beam x-ray sources

    CERN Document Server

    Failor, B H; Riordan, j c; Lojewski, D Y

    2007-01-01

    High power x-ray sources built for nuclear weapons effects testing are evolving toward larger overall diameters and smaller anode cathode gaps. We describe a framing camera developed to measure the time-evolution of these 20-50 ns pulsed x-ray sources produced by currents in the 1.5-2.5 MA range and endpoint voltages between 0.2 and 1.5 MV. The camera has up to 4 frames with 5 ns gate widths; the frames are separated by 5 ns. The image data are recorded electronically with a gated intensified CCD camera and the data are available immediately following a shot. A fast plastic scintillator (2.1 ns decay time) converts the x-rays to visible light and, for high sensitivity, a fiber optic imaging bundle carries the light to the CCD input. Examples of image data are shown.

  1. Electron localization in fragmentation of H{sub 2} with CEP stabilized laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Kremer, Manuel; Fischer, Bettina; Feuerstein, Bernold; Sharma, Vandana; Hofrichter, Christian; Schroeter, Claus Dieter; Moshammer, Robert [Max-Planck-Institut fuer Kernphysik, Heidelberg (Germany); Jesus, Vitor L.B. de [Instituto Federal de Educacao, Ciencia e Tecnologia do Rio de Janeiro (IFRJ), Nilopolis, RJ (Brazil); Rudenko, Artem [Max-Planck Advanced Study Group, CFEL, Hamburg (Germany); Thumm, Uwe [James R. Macdonald Laboratory, Kansas State University, Manhattan, Kansas (United States)

    2010-07-01

    Fully differential data for H{sub 2} dissociation in ultrashort (6fs, 760 nm), linearly polarized, intense (0.44 PW/cm{sup 2}) laser pulses with a stabilized carrier-envelope phase (CEP) were recorded with a reaction microscope. Depending on the CEP, the molecular orientation, and the kinetic energy release (KER), we see a clear asymmetry in the proton emission for kinetic energy releases between 0-3 eV as basically predicted by Roudnev and Esry and much stronger than in earlier measurements by Kling et al. Wave packet propagation simulations were carried out, which reproduce the salient features and together with the KER-independent electron asymmetry observed in the experiment, rule out the first ionization step to be the reason for the asymmetric proton emission.

  2. High efficiency DNA delivery into swine oocytes and embryos by electronic pulse delivery (EPD).

    Science.gov (United States)

    Yang, Y; Huang, S H; Zhao, X

    1997-06-01

    The production of transgenic swine for xenotransplantation has been proposed as an optimal option to overcome the chronic shortage of human organ donors. Generation of genetically engineered swine has been elusive due to the difficulties in gene transfer. In order to achieve effective gene delivery, a key step for the genetic modification, we applied electronic pulse delivery (EPD) technology to introduce H2Kb-DC DNA construct into swine eggs. Using the developed EPD Protocols, we have achieved good viability of the EPD treated oocytes, satisfactory embryonic development of the EPD treated embryos, and stable DNA transfer into the swine embryos with high efficiency. Thus, application of the EPD technology promises to effectively facilitate the generation of large transgenic mammals.

  3. Reaction of a hydrated electron with gentamycin and collagen—A pulse radiolysis study

    Science.gov (United States)

    Pietrucha, K.; Góra, L.; Doillon, C. J.

    1996-01-01

    The reactions of a hydrated electron (e aq-) with aminoglycoside anbiotic gentamycin and collagen in aqueous medium at different pH have been investigated employing a pulse radiolysis technique. The pseudo-first order equation of reaction kinetics was used to give an accurate description of the decay of e aq- in gentamycin solutions. The rate constant of the e aq- decay in collagen solution was high and reached 3.2 × 10 10 M -1 s -1. The rate constants for the reaction of the e aq- with gentamycin were found to be influenced by pH, decreasing with the deprotonation of the -NH 3 groups, while for pH > pK a which for gentamycin is equal to 7.8, the rate constant was unchanged. These observations suggest that when the amino groups are protonated, reductive deamination occurs, but for unprotonated non-reactive amino groups, a radical anion is formed on the glycoside moiety.

  4. Size-dependent ultrafast ionization dynamics of nanoscale samples in intense femtosecond x-ray free-electron-laser pulses.

    Science.gov (United States)

    Schorb, Sebastian; Rupp, Daniela; Swiggers, Michelle L; Coffee, Ryan N; Messerschmidt, Marc; Williams, Garth; Bozek, John D; Wada, Shin-Ichi; Kornilov, Oleg; Möller, Thomas; Bostedt, Christoph

    2012-06-08

    All matter exposed to intense femtosecond x-ray pulses from the Linac Coherent Light Source free-electron laser is strongly ionized on time scales competing with the inner-shell vacancy lifetimes. We show that for nanoscale objects the environment, i.e., nanoparticle size, is an important parameter for the time-dependent ionization dynamics. The Auger lifetimes of large Ar clusters are found to be increased compared to small clusters and isolated atoms, due to delocalization of the valence electrons in the x-ray-induced nanoplasma. As a consequence, large nanometer-sized samples absorb intense femtosecond x-ray pulses less efficiently than small ones.

  5. Attosecond angular flux of partial charges on the carbon atoms of benzene in non-aromatic excited state

    Science.gov (United States)

    Hermann, Gunter; Liu, ChunMei; Manz, Jörn; Paulus, Beate; Pohl, Vincent; Tremblay, Jean Christophe

    2017-09-01

    Recently, it was discovered that excitation of the oriented model benzene from its aromatic electronic ground state S0 (1A1g) to the non-aromatic S0 +S2 (1B1u) superposition state generates negative and positive partial charges on alternating carbon atoms. Subsequently, they vary periodically, due to adiabatic attosecond charge migration AACM. Here, we determine the angular electronic flux that mediates this new type of AACM, by means of quantum dynamics simulations. It is found to be periodic, with period τ bar = 590as , and with a pincer motion type pattern such that a total of 1.2 valence electrons flow concertedly between alternating sources and sinks at the carbon nuclei.

  6. Integrated testing of the Thales LPT9510 pulse tube cooler and the iris LCCE electronics

    Science.gov (United States)

    Johnson, Dean L.; Rodriguez, Jose I.; Carroll, Brian A.; Bustamante, John G.; Kirkconnell, Carl S.; Luong, Thomas T.; Murphy, J. B.; Haley, Michael F.

    2014-01-01

    The Jet Propulsion Laboratory (JPL) has identified the Thales LPT9510 pulse tube cryocooler as a candidate low cost cryocooler to provide active cooling on future cost-capped scientific missions. The commercially available cooler can provide refrigeration in excess of 2 W at 100K for 60W of power. JPL purchased the LPT9510 cooler for thermal and dynamic performance characterization, and has initiated the flight qualification of the existing cooler design to satisfy near-term JPL needs for this cooler. The LPT9510 has been thermally tested over the heat reject temperature range of 0C to +40C during characterization testing. The cooler was placed on a force dynamometer to measure the selfgenerated vibration of the cooler. Iris Technology has provided JPL with a brass board version of the Low Cost Cryocooler Electronics (LCCE) to drive the Thales cooler during characterization testing. The LCCE provides precision closed-loop temperature control and embodies extensive protection circuitry for handling and operational robustness; other features such as exported vibration mitigation and low frequency input current filtering are envisioned as options that future flight versions may or may not include based upon the mission requirements. JPL has also chosen to partner with Iris Technology for the development of electronics suitable for future flight applications. Iris Technology is building a set of radiation-hard, flight-design electronics to deliver to the Air Force Research Laboratory (AFRL). Test results of the thermal, dynamic and EMC testing of the integrated Thales LPT9510 cooler and Iris LCCE electronics is presented here.

  7. Surface modification of 40CrNiMo7 steel with high current pulsed electron beam treatment

    Science.gov (United States)

    Hao, Shengzhi; Wang, Huihui; Zhao, Limin

    2016-02-01

    High current pulsed electron beam (HCPEB) treatment was conducted on 40CrNiMo7 steel with accelerating voltage 27 kV, energy density 3 J/cm2, pulse duration 2.5 μs and 1-50 pulses. The evolutions of surface microstructure were investigated by using optical microscopy (OM), X-ray diffraction (XRD), scanning electron microscope (SEM) and transmission electron microscopy (TEM) techniques. It was found that the carbides in the surface remelted layer of depth ∼4 μm were dissolved gradually along with the increasing number of HCPEB pulses. Eventually, the surface microstructure of 40CrNiMo7 steel was transformed to a complex structure composed of very refined ∼150 nm austenite as the main part and a little quantity of martensite phases. After 15 pulses of HCPEB treatment, the surface microhardness was doubled to 553 HV, and the wear rate decreased to one third of the initial state correspondingly.

  8. Effect of gas heating on the generation of an ultrashort avalanche electron beam in the pulse-periodic regime

    Science.gov (United States)

    Baksht, E. Kh.; Burachenko, A. G.; Lomaev, M. I.; Sorokin, D. A.; Tarasenko, V. F.

    2015-07-01

    The generation of an ultrashort avalanche electron beam (UAEB) in nitrogen in the pulse-periodic regime is investigated. The gas temperature in the discharge gap of the atmospheric-pressure nitrogen is measured from the intensity distribution of unresolved rotational transitions ( C 3Π u , v' = 0) → ( B 3Π g , v″ = 0) in the nitrogen molecule for an excitation pulse repetition rate of 2 kHz. It is shown that an increase in the UAEB current amplitude in the pulse-periodic regime is due to gas heating by a series of previous pulses, which leads to an increase in the reduced electric field strength as a result of a decrease in the gas density in the zone of the discharge formation. It is found that in the pulse-periodic regime and the formation of the diffuse discharge, the number of electrons in the beam increases by several times for a nitrogen pressure of 9 × 103 Pa. The dependences of the number of electrons in the UAEB on the time of operation of the generator are considered.

  9. Interaction of short x-ray pulses with low-Z x-ray optics materials at the LCLS free-electron laser

    NARCIS (Netherlands)

    Hau-Riege, S. P.; London, R. A.; Graf, A.; Baker, S. L.; Soufli, R.; Sobierajski, R.; Burian, T.; Chalupsky, J.; Juha, L.; Gaudin, J.; Krzywinski, J.; Moeller, S.; Messerschmidt, M.; Bozek, J.; Bostedt, C.

    2010-01-01

    Materials used for hard x-ray-free-electron laser (XFEL) optics must withstand high-intensity x-ray pulses. The advent of the Linac Coherent Light Source has enabled us to expose candidate optical materials, such as bulk B4C and SiC films, to 0.83 keV XFEL pulses with pulse energies between 1 mu J

  10. Measurement of the single-shot pulse energy of a free electron laser using a cryogenic radiometer

    Energy Technology Data Exchange (ETDEWEB)

    Masahiro, Kato; Norio, Saito; Yuichiro, Morishita; Takahiro, Tanaka [National Institute of Advanced Industrial Science and Technology (AIST), NMIJ, Tsukuba (Japan); Masahiro, Kato; Norio, Saito; Kai, Tiedtke; Pavle N, Juranic; Sorokin, A.A.; Richter, M.; Takahiro, Tanaka; Mitsuru, Nagasono; Makina, Yabashi; Kensuke, Tono; Tadashi, Togashi; Tetsuya, Ishikawa [RIKEN, XFEL Project Head Office, Kouto, Sayo, Hyogo (Japan); Kai, Tiedtke; Pavle N, Juranic; Sorokin, A.A.; Jastrow, U. [Deutsches Elektronen-Synchrotron, DESY, Hamburg (Germany); Sorokin, A.A. [Ioffe Physico-Technical Institute, Polytekhnicheskaya 26, St Petersburg (Russian Federation); Richter, M.; Kroth, U.; Schoppe, H. [Physikalisch-Technische Bundesanstalt, PTB, Berlin (Germany); Tadashi, Togashi; Hiroaki, Kimura; Haruhiko, Ohashi [Japan Synchrotron Radiation Research Institute, Sayo, Hyogo (Japan)

    2010-10-15

    The absolute single-shot pulse energy of the SPring 8 extreme ultraviolet (EUV) free electron laser (FEL) was measured using a cryogenic radiometer with a relative standard uncertainty of 3%. The temperature change of the cavity in the cryogenic radiometer caused by an incident FEL pulse was determined using a lock-in amplifier and an ac Wheatstone bridge. The measured pulse energies were compared with a gas-monitor detector developed by Physikalisch-Technische Bundesanstalt/Deutsches Elektronen-Synchrotron/Ioffe Physico-Technical Institute (Ioffe) at a wavelength of 51.3 nm at the SPring-8 EUV-FEL in a shot-to-shot mode. The pulse energies measured using the two detectors agree within 2.0%. (authors)

  11. Large Pulsed Electron Beam Welded Percolation Networks of Silver Nanowires for Transparent and Flexible Electrodes.

    Science.gov (United States)

    Kim, Jisoo; Nam, Yun Seok; Song, Myoung Hoon; Park, Hyung Wook

    2016-08-17

    Mechanical properties of transparent electrodes, including flexibility, are important in flexible electronics for sustaining electrical conductivity under bending with small radius of curvature. Low contact resistance of junctions in metal nanowire percolation networks is the most important factor to produce electrodes with excellent optical, electrical and mechanical performance. Here, we report the fabrication of welded silver nanowire percolation networks using large pulsed electron beam (LPEB) irradiation as a welding process of silver nanowires (AgNWs). It results in modification of electrical and mechanical properties because of the low contact resistance at welded junctions. Consequently, the flexible and transparent AgNW electrodes fabricated by LPEB irradiation showed lower sheet resistance of 12.63 Ω sq(-1) at high transmittance of 93% (at 550 nm), and superb mechanical flexibility, compared with other AgNW electrodes prepared by thermal treatement and without any treatment. Polymer light-emitting diodes (PLEDs) using AgNWs by LPEB irradiation were fabricated to confirm that the AgNW electrode by LPEB irradiation was able to become alternative to indium tin oxide (ITO) and they showed good device performance as a maximum luminous efficiency of 7.37 cd A(-1), and excellent mechanical flexibility under bending with small radius of curvature.

  12. Short-pulse, high-energy radiation generation from laser-wakefield accelerated electron beams

    Science.gov (United States)

    Schumaker, Will

    2013-10-01

    Recent experimental results of laser wakefield acceleration (LWFA) of ~GeV electrons driven by the 200TW HERCULES and the 400TW ASTRA-GEMINI laser systems and their subsequent generation of photons, positrons, and neutrons are presented. In LWFA, high-intensity (I >1019 W /cm2), ultra-short (τL counter-propagating, ultra-high intensity (I >1021 W /cm2) laser pulse to undergo inverse Compton scattering and emit a high-peak brightness beam of high-energy photons. Preliminary results and experimental sensitivities of the electron-laser beam overlap are presented. The high-energy photon beams can be spectrally resolved using a forward Compton scattering spectrometer. Moreover, the photon flux can be characterized by a pixelated scintillator array and by nuclear activation and (γ,n) neutron measurements from the photons interacting with a secondary solid target. Monte-Carlo simulations were performed using FLUKA to support the yield estimates. This research was supported by DOE/NSF-PHY 0810979, NSF CAREER 1054164, DARPA AXiS N66001-11-1-4208, SF/DNDO F021166, and the Leverhulme Trust ECF-2011-383.

  13. Intense Far-Infrared Free-Electron Laser-Pulses with a Length of 6 Optical Cycles

    NARCIS (Netherlands)

    Knippels, G.M.H.; R F X A M Mols,; van der Meer, A. F. G.; Oepts, D.; van Amersfoort, P. W.

    1995-01-01

    Second-order optical autocorrelation measurements are reported for a far-infrared free-electron laser. Second-harmonic generation in an 840-mu m-long CdTe crystal is used to provide the nonlinear autocorrelation signal. At wavelengths of 10.4 and 24.5 mu m, FWHM pulse durations of 220 and 500 fs,

  14. Design and simulation of laser wakefield acceleration with external electron bunch injection in front of the laser pulse

    NARCIS (Netherlands)

    Irman, A.; Luttikhof, M.J.H.; Khachatryan, A.G.; van Goor, F.A.; Verschuur, Jeroen W.J.; Bastiaens, Hubertus M.J.; Boller, Klaus J.

    2007-01-01

    In this article we present a theoretical investigation on an experimental design of a laser wakefield accelerator in which electron bunches from a photocathode radio frequency linac are injected into a capillary discharge plasma channel just in front of a few tens of terawatt drive laser pulse. The

  15. Pulsed electron beam propagation in gases under pressure of 6.6 kPa in drift tube

    Energy Technology Data Exchange (ETDEWEB)

    Kholodnaya, G.E., E-mail: galina_holodnaya@mail.ru; Sazonov, R.V.; Ponomarev, D.V.; Remnev, G.E.; Poloskov, A.V.

    2017-02-01

    This paper presents the results of an investigation of pulsed electron beam transport propagated in a drift tube filled with different gases (He, H{sub 2}, N{sub 2}, Ar, SF{sub 6}, and CO{sub 2}). The total pressure in the drift tube was 6.6 kPa. The experiments were carried out using a TEA-500 pulsed electron accelerator. The electron beam was propagated in the drift tube composed of two sections equipped with reverse current shunts. Under a pressure of 6.6 kPa, the maximum value of the electron beam charge closed on the walls of the drift tube was recorded when the beam was propagated in hydrogen and carbon dioxide. The minimum value of the electron beam charge closed on the walls of the drift tube was recorded for sulfur hexafluoride. The visualization of the pulsed electron beam energy losses onto the walls of the drift chamber was carried out using radiation-sensitive film.

  16. Pulsed field ionization electron spectroscopy and molecular structure of aluminum uracil.

    Science.gov (United States)

    Krasnokutski, Serge A; Yang, Dong-Sheng

    2007-10-25

    Al-uracil (Al-C4H4N2O2) was synthesized in a laser-vaporization supersonic molecular beam source and studied with pulsed field ionization-zero electron kinetic energy (ZEKE) photoelectron spectroscopy and density functional theory (DFT). The DFT calculations predicted several low-energy Al-uracil isomers with Al binding to the diketo, keto-enol, and dienol tautomers of uracil. The ZEKE spectroscopic measurements of Al-uracil determined the ionization energy of 43 064(5) cm-1 [or 5.340(6) eV] and a vibrational mode of 51 cm-1 for the neutral complex and several vibrational modes of 51, 303, 614, and 739 cm-1 for the ionized species. Combination of the ZEEK spectrum with the DFT and Franck-Condon factor calculations determined the preferred isomeric structure and electronic states of the Al-uracil complex. This isomer is formed by Al binding to the O4 atom of the diketo tautomer of uracil and has a planar Cs symmetry. The ground electronic states of the neutral and ionized species are 2A' ' and 1A', respectively. The 2A' ' neutral state has a slightly shorter Al-O4 distance than the 1A' ion state. However, the 1A' ion state has stronger metal-ligand binding compared to the 2A' ' state. The increased Al-O4 distance from the 2A' ' state to the 1A' state is attributed to the loss of the pi binding interaction between Al and O4 in the singlet ion state, whereas the increased metal-ligand binding strength is due to the additional charge-dipole interaction in the ion that surpasses the loss of the pi orbital interaction.

  17. Propagation of intense and short circularly polarized pulses in a molecular gas: From multiphoton ionization to nonlinear macroscopic effects

    Science.gov (United States)

    Lytova, M.; Lorin, E.; Bandrauk, A. D.

    2016-07-01

    We present a detailed analysis of the propagation dynamics of short and intense circularly polarized pulses in an aligned diatomic gas. Compared to linearly polarized intense pulses, high harmonic generation (HHG) and the coherent generation of attosecond pulses in the intense-circular-polarization case are a new research area. More specifically, we numerically study the propagation of intense and short circularly polarized pulses in the one-electron H2+ molecular gas, using a micro-macro Maxwell-Schrödinger model. In this model, the macroscopic polarization is computed from the solution of a large number of time-dependent Schrödinger equations, the source of dipole moments, and using a trace operator. We focus on the intensity and the phase of harmonics generated in the H2+ gas as a function of the pulse-propagation distance. We show that short coherent circularly polarized pulses of same helicity can be generated in the molecular gas as a result of cooperative phase-matching effects.

  18. New theoretical approaches to atomic and molecular dynamics triggered by ultrashort light pulses on the atto- to picosecond time scale

    Energy Technology Data Exchange (ETDEWEB)

    Pabst, Stefan Ulf

    2013-04-15

    The concept of atoms as the building blocks of matter has existed for over 3000 years. A revolution in the understanding and the description of atoms and molecules has occurred in the last century with the birth of quantum mechanics. After the electronic structure was understood, interest in studying the dynamics of electrons, atoms, and molecules increased. However, time-resolved investigations of these ultrafast processes were not possible until recently. The typical time scale of atomic and molecular processes is in the picosecond to attosecond realm. Tremendous technological progress in recent years makes it possible to generate light pulses on these time scales. With such ultrashort pulses, atomic and molecular dynamics can be triggered, watched, and controlled. Simultaneously, the need rises for theoretical models describing the underlying mechanisms. This doctoral thesis focuses on the development of theoretical models which can be used to study the dynamical behavior of electrons, atoms, and molecules in the presence of ultrashort light pulses. Several examples are discussed illustrating how light pulses can trigger and control electronic, atomic, and molecular motions. In the first part of this work, I focus on the rotational motion of asymmetric molecules, which happens on picosecond and femtosecond time scales. Here, the aim is to align all three axes of the molecule as well as possible. To investigate theoretically alignment dynamics, I developed a program that can describe alignment motion ranging from the impulsive to the adiabatic regime. The asymmetric molecule SO{sub 2} is taken as an example to discuss strategies of optimizing 3D alignment without the presence of an external field (i.e., field-free alignment). Field-free alignment is particularly advantageous because subsequent experiments on the aligned molecule are not perturbed by the aligning light pulse. Wellaligned molecules in the gas phase are suitable for diffraction experiments. From the

  19. Flexible control of femtosecond pulse duration and separation using an emittance-spoiling foil in x-ray free-electron lasers

    Energy Technology Data Exchange (ETDEWEB)

    Ding, Y. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Behrens, C. [Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Coffee, R. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Decker, F. -J. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Emma, P. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Field, C. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Helml, W. [Technische Univ. Munchen, Garching (Germany); Huang, Z. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Krejcik, P. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Krzywinski, J. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Loos, H. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Lutman, A. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Marinelli, A. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Maxwell, T. J. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Turner, J. [SLAC National Accelerator Lab., Menlo Park, CA (United States)

    2015-06-22

    We report experimental studies of generating and controlling femtosecond x-ray pulses in free-electron lasers (FELs) using an emittance spoiling foil. By selectivity spoiling the transverse emittance of the electron beam, the output pulse duration or double-pulse separation is adjusted with a variable size single or double slotted foil. Measurements were performed with an X-band transverse deflector located downstream of the FEL undulator, from which both the FEL lasing and emittance spoiling effects are observed directly.

  20. Halo Evolution of Hypereutectic Al-17.5Si Alloy Treated with High-Current Pulsed Electron Beam

    Directory of Open Access Journals (Sweden)

    L. Hu

    2015-01-01

    Full Text Available Halo evolution of an Al-17.5Si alloy surface after treatment with increasing pulse numbers of a high-current pulsed electron beam (HCPEB was investigated. A halo is a ring microstructure resembling a bull’s eye. SEM results indicate that the nanocrystallization of halo induced by HCPEB treatment leads to gradual diffusion of the Si phase. Multiple pulses numbers cause the Si phase to be significantly refined and uniformly distributed. In addition, nanosilicon particles with a grain size of 30~100 nm were formed after HCPEB treatment, as shown by TEM observation. XRD results indicate that Si diffraction peaks broadened after HCPEB treatment. The microhardness tests demonstrate that the microhardness at the midpoint from the halo edge to center decreased sharply from 9770.7 MPa at 5 pulses to 2664.14 MPa at 25 pulses. The relative wear resistance of a 15-pulse sample is effectively improved by a factor of 6.5, exhibiting optimal wear resistance.

  1. Improving the output voltage waveform of an intense electron-beam accelerator based on helical type Blumlein pulse forming line

    Directory of Open Access Journals (Sweden)

    Xin-Bing Cheng

    2010-07-01

    Full Text Available The Blumlein pulse forming line (BPFL consisting of an inner coaxial pulse forming line (PFL and an outer coaxial PFL is widely used in the field of pulsed power, especially for intense electron-beam accelerators (IEBA. The output voltage waveform determines the quality and characteristics of the output beam current of the IEBA. Comparing with the conventional BPFL, an IEBA based on a helical type BPFL can increase the duration of the output voltage in the same geometrical volume. However, for the helical type BPFL, the voltage waveform on a matched load may be distorted which influences the electron-beam quality. In this paper, an IEBA based on helical type BPFL is studied theoretically. Based on telegrapher equations of the BPFL, a formula for the output voltage of IEBA is obtained when the transition section is taken into account, where the transition section is between the middle cylinder of BPFL and the load. From the theoretical analysis, it is found that the wave impedance and transit time of the transition section influence considerably the main pulse voltage waveform at the load, a step is formed in front of the main pulse, and a sharp spike is also formed at the end of the main pulse. In order to get a well-shaped square waveform at the load and to improve the electron-beam quality of such an accelerator, the wave impedance of the transition section should be equal to that of the inner PFL of helical type BPFL and the transit time of the transition section should be designed as short as possible. Experiments performed on an IEBA with the helical type BPFL show reasonable agreement with theoretical analysis.

  2. Large-charge quasimonoenergetic electron beams produced by off-axis colliding laser pulses in underdense plasma

    Science.gov (United States)

    Deng, Z. G.; Zhang, Z. M.; Zhang, B.; He, S. K.; Teng, J.; Hong, W.; Dong, K. G.; Wu, Y. C.; Zhu, B.; Gu, Y. Q.

    2017-02-01

    Electrons can be efficiently injected into a plasma wave by colliding two counterpropagating laser pulses in a laser wakefield acceleration. However, the generation of a high-quality electron beam with a large charge is difficult in the traditional on-axis colliding scheme due to the growth of the electron beam duration coming from the increase of the beam charge. To solve this problem, we propose an off-axis colliding scheme, in which the collision point is away from the axis of the driver pulse. We show that the electrons injected from the off-axis region are highly concentered on the tail of the bubble even for a large trapped charge, thus feeling almost the same accelerating field. As a result, quasimonoenergetic electron beams with a large charge can be produced. The validity of this scheme is confirmed by both the particle-in-cell simulations and the Hamiltonian model. Furthermore, it is shown that a Laguerre-Gauss (LG) laser can be adopted as the injection pulse to realize the off-axis colliding injection in three dimensions symmetrically, which may be useful in simplifying the technical layout of the real experiment setup.

  3. A battery-operated, stabilized, high-energy pulsed electron gun for the production of rare gas excimers.

    Science.gov (United States)

    Barcellan, L; Berto, E; Carugno, G; Galet, G; Galeazzi, G; Borghesani, A F

    2011-09-01

    We report on the design of a new type of hot-filament electron gun delivering fairly high current (a few hundreds of μ A) at high voltage (up to 100 kV) in continuous or pulsed mode. Its novel features are that the filament is heated by means of a pack of rechargeable batteries floated atop the high-voltage power supply in order to get rid of bulky isolation transformers, and that the filament current and, hence, the electron gun current, is controlled by a feedback circuit including a superluminescent diode decoupled from the high voltage by means of an optical fiber. This electron gun is intended for general purposes, although we have especially developed it to meet the needs of our experiment on the infrared emission spectroscopy of rare gas excimers. Our experiment requires that the charge injection into the sample is pulsed and constant and stable in time. The new electron gun can deliver several tens of nC per pulse of electrons of energy up to 100 keV into the sample cell. The new design also eliminates ripples in the emission current and ensures up to 12 h of stable performance. © 2011 American Institute of Physics

  4. Nonlinear Dichroism in Back-to-Back Double Ionization of He by an Intense Elliptically Polarized Few-Cycle Extreme Ultraviolet Pulse.

    Science.gov (United States)

    Ngoko Djiokap, J M; Manakov, N L; Meremianin, A V; Hu, S X; Madsen, L B; Starace, Anthony F

    2014-11-28

    Control of double ionization of He by means of the polarization and carrier-envelope phase (CEP) of an intense, few-cycle extreme ultraviolet (XUV) pulse is demonstrated numerically by solving the six-dimensional two-electron, time-dependent Schrödinger equation for He interacting with an elliptically polarized XUV pulse. Guided by perturbation theory (PT), we predict the existence of a nonlinear dichroic effect (∝I^{3/2}) that is sensitive to the CEP, ellipticity, peak intensity I, and temporal duration of the pulse. This dichroic effect (i.e., the difference of the two-electron angular distributions for opposite helicities of the ionizing XUV pulse) originates from interference of first- and second-order PT amplitudes, allowing one to probe and control S- and D-wave channels of the two-electron continuum. We show that the back-to-back in-plane geometry with unequal energy sharing is an ideal one for observing this dichroic effect that occurs only for an elliptically polarized, few-cycle attosecond pulse.

  5. Coherent Multidimensional Core Spectroscopy of Molecules with Multiple X-ray pulses

    Science.gov (United States)

    Mukamel, Shaul

    2017-04-01

    Multidimensional spectroscopy uses sequences of optical pulses to study dynamical processes in complex molecules through correlation plots involving several time delay periods. Extensions of these techniques to the x-ray regime will be discussed. Ultrafast nonlinear x-ray spectroscopy is made possible by newly developed free electron laser and high harmonic generation sources. The attosecond duration of X-ray pulses and the atomic selectivity of core X-ray excitations offer a uniquely high spatial and temporal resolution. We demonstrate how stimulated Raman detection of an X-ray probe may be used to monitor the phase and dynamics of the nonequilibrium valence electronic state wavepacket created by e.g. photoexcitation, photoionization and Auger processes. Spectroscopy of multiplecore excitations provides a new window into electron correlations. Applications will be presented to long-range charge transfer in proteins and to excitation energy transfer in porphyrin arrays. Conical intersections (CoIn) dominate the pathways and outcomes of virtually all photophysical and photochemical molecular processes. Despite extensive experimental and theoretical effort CoIns have not been directly observed yet and the experimental evidence is being inferred from fast reaction rates and some vibrational signatures. Novel ultrafast X ray probes for these processes will be presented. Short X-ray pulses can directly detect the passage through a CoIn with the adequate temporal and spectral sensitivity. The technique is based on a coherent Raman process that employs a composite femtosecond/attosecond X-ray pulse to directly detect the electronic coherences (rather than populations) that are generated as the system passes through the CoIn. Streaking of time-resolved photoelectron spectroscopy (TRPES) signals offers another powerful window into the joint electronic/vibrational dynamics at concial intersections. Strong coupling of molecules to the vacuum field of micro cavities can modify

  6. Improving corrosion and wear resistance of FV520B steel by high current pulsed electron beam surface treatment

    Energy Technology Data Exchange (ETDEWEB)

    Hao, Shengzhi, E-mail: ebeam@dlut.edu.cn [Key Laboratory of Material Modification by Laser, Ion and Electron Beams, Ministry of Education, Dalian University of Technology, Dalian 116024 (China); Zhao, Limin [School of Materials Science and Engineering, Dalian Jiaotong University, Dalian 116028 (China); Zhang, Yanlong; Wang, Huihui [Key Laboratory of Material Modification by Laser, Ion and Electron Beams, Ministry of Education, Dalian University of Technology, Dalian 116024 (China)

    2015-08-01

    Highlights: • HCPEB surface treatment was conducted on FV520B steel. • Surface layer ∼10 μm was refined with elements homogenization. • Remelted layer exhibited 〈2 0 0〉 preferential orientation. • Corrosion potential increased and corrosion rate decreased one order of magnitude. • Wear resistance increased by 3 times. - Abstract: High current pulsed electron beam (HCPEB) surface treatment was conducted on FV520B steel with accelerating voltage 27 kV, pulse duration 2.5 μs, energy density 5 J/cm{sup 2} and 1–25 pulses. The surface microstructure and element distribution were examined by using scanning electron microscope (SEM), electron probe micro-analysis (EPMA) and X-ray diffraction (XRD) methods. After HCPEB treatments, the surface microstructure became refined and uniform with an average grain size less than 2 μm and a preferential solidification orientation in 〈2 0 0〉 direction. The thickness of surface remelted layer was ∼4 μm. The initial precipitated particles in surface layer of depth ∼10 μm were dissolved into the base matrix and gave a homogenous element distribution. The HCPEB modified surface exhibited an effective improvement in corrosion and wear resistance. The corrosion potential shifted towards positive and the corrosion rate decreased nearly one order of magnitude, while the wear resistance after 25 pulses of HCPEB treatment increased by 3 times as compared with the initial FV520B steel.

  7. Distance dependence of the reaction rate for the reduction of metal cations by solvated electrons: a picosecond pulse radiolysis study.

    Science.gov (United States)

    Schmidhammer, Uli; Pernot, Pascal; De Waele, Vincent; Jeunesse, Pierre; Demarque, Alexandre; Murata, Shigeo; Mostafavi, Mehran

    2010-11-18

    The decay of the solvated electron generated by picosecond electron pulse radiolysis is studied by broad-band transient absorption measurements in ethylene glycol solutions containing decimolar concentrations of Cu(2+), Ni(2+), and Pb(2+) metal cations. Analysis of the nonexponential kinetics of the decays reveals molecular parameters of the electron transfer reaction. It is found that the reaction occurs at long distance for Cu(2+) solutions and is only limited to contact distance in the case of Ni(2+) solutions. The distribution of reaction distance strongly depends on the free enthalpy change of the reactions.

  8. Reaction of a hydrated electron with gentamycin and collagen -a pulse radiolysis study

    Energy Technology Data Exchange (ETDEWEB)

    Pietrucha, K. [Technical Univ., Lodz (Poland). Inst. of Applied Radiation Chemistry; Gora, L. [Worcester Poltechnic Inst., MA (United States). Dept. of Chemical Engineering; Doillon, C.J. [Laval Univ., Quebec, PQ (Canada). Dept. of Surgery]|[Saint-Francois d`Assise Hospital, Quebec (Canada)

    1996-01-01

    The reactions of a hydrated electron (e{sub aq}{sup -}) with aminoglycoside antibiotic gentamycin and collagen in aqueous medium at different pH have been investigated employing a pulse radiolysis technique. The pseudo-first order equation of reaction kinetics was used to give an accurate description of the decay of e{sub aq}{sup -} in gentamycin solutions. The rate constant of the e{sub aq}{sup -}decay in collagen solutions was high and reached 3.2 x 10{sup 10} M{sup -1} s{sup -1}. The rate constants for the reaction of the e{sub aq}{sup -}with gentamycin were found to be influenced by pH, decreasing with the deprotonation of the -NH{sub 3} groups, while for pH > pK{sub a} which for gentamycin is equal to 7.8, the rate constant was unchanged. These observations suggest that when the amino groups are protonated, reductive deamination occurs, but for unprotonated non-reactive amino groups, a radical anion is formed on the glycoside moiety. (Author).

  9. High energy micro electron beam generation using chirped laser pulse in the presence of an axial magnetic field

    Science.gov (United States)

    Akou, H.; Hamedi, M.

    2015-10-01

    In this paper, the generation of high-quality and high-energy micro electron beam in vacuum by a chirped Gaussian laser pulse in the presence of an axial magnetic field is numerically investigated. The features of energy and angular spectra, emittances, and position distribution of electron beam are compared in two cases, i.e., in the presence and absence of an external magnetic field. The electron beam is accelerated with higher energy and qualified in spatial distribution in the presence of the magnetic field. The presence of an axial magnetic field improves electron beam spatial quality as well as its gained energy through keeping the electron motion parallel to the direction of propagation for longer distances. It has been found that a 64 μm electron bunch with about MeV initial energy becomes a 20 μm electron beam with high energy of the order of GeV, after interacting with a laser pulse in the presence of an external magnetic field.

  10. High energy micro electron beam generation using chirped laser pulse in the presence of an axial magnetic field

    Energy Technology Data Exchange (ETDEWEB)

    Akou, H., E-mail: h.akou@nit.ac.ir; Hamedi, M. [Department of Physics, Faculty of Basic Science, Babol University of Technology, Babol 47148-71167 (Iran, Islamic Republic of)

    2015-10-15

    In this paper, the generation of high-quality and high-energy micro electron beam in vacuum by a chirped Gaussian laser pulse in the presence of an axial magnetic field is numerically investigated. The features of energy and angular spectra, emittances, and position distribution of electron beam are compared in two cases, i.e., in the presence and absence of an external magnetic field. The electron beam is accelerated with higher energy and qualified in spatial distribution in the presence of the magnetic field. The presence of an axial magnetic field improves electron beam spatial quality as well as its gained energy through keeping the electron motion parallel to the direction of propagation for longer distances. It has been found that a 64 μm electron bunch with about MeV initial energy becomes a 20 μm electron beam with high energy of the order of GeV, after interacting with a laser pulse in the presence of an external magnetic field.

  11. Analysis of the damage threshold of the GaAs pseudomorphic high electron mobility transistor induced by the electromagnetic pulse

    Science.gov (United States)

    Xi, Xiao-Wen; Chai, Chang-Chun; Liu, Yang; Yang, Yin-Tang; Fan, Qing-Yang; Shi, Chun-Lei

    2016-08-01

    An electromagnetic pulse (EMP)-induced damage model based on the internal damage mechanism of the GaAs pseudomorphic high electron mobility transistor (PHEMT) is established in this paper. With this model, the relationships among the damage power, damage energy, pulse width and signal amplitude are investigated. Simulation results show that the pulse width index from the damage power formula obtained here is higher than that from the empirical formula due to the hotspot transferring in the damage process of the device. It is observed that the damage energy is not a constant, which decreases with the signal amplitude increasing, and then changes little when the signal amplitude reaches up to a certain level. Project supported by the National Basic Research Program of China (Grant No. 2014CB339900) and the Open Fund of Key Laboratory of Complex Electromagnetic Environment Science and Technology, China Academy of Engineering Physics (CAEP) (Grant No. 2015-0214.XY.K).

  12. Mathematical modeling of the infrastructure of attosecond actuators and femtosecond sensors of nonequilibrium physical media in smart materials

    Science.gov (United States)

    Beznosyuk, Sergey A.; Maslova, Olga A.; Zhukovsky, Mark S.; Valeryeva, Ekaterina V.; Terentyeva, Yulia V.

    2017-12-01

    The task of modeling the multiscale infrastructure of quantum attosecond actuators and femtosecond sensors of nonequilibrium physical media in smart materials is considered. Computer design and calculation of supra-atomic femtosecond sensors of nonequilibrium physical media in materials based on layered graphene-transition metal nanosystems are carried out by vdW-DF and B3LYP methods. It is shown that the molybdenum substrate provides fixation of graphene nanosheets by Van der Waals forces at a considerable distance (5.3 Å) from the metal surface. This minimizes the effect of the electronic and nuclear subsystem of the substrate metal on the sensory properties of "pure" graphene. The conclusion is substantiated that graphene-molybdenum nanosensors are able to accurately orient and position one molecule of carbon monoxide. It is shown that graphene selectively adsorbs CO and fixes the oxygen atom of the molecule at the position of the center of the graphene ring C6.

  13. Transmission electron microscopy studying of structural features of NiTi B2 phase formed under pulsed electron-beam impact

    Energy Technology Data Exchange (ETDEWEB)

    Meisner, Ludmila L.; Semin, Viktor O.; Gudimova, Ekaterina Y. [Institute of Strength Physicists and Materials Science SB RAS, Tomsk, 634055 (Russian Federation); National Research Tomsk State University, Tomsk, 634050 (Russian Federation); Neiman, Alexey A., E-mail: nasa@ispms.tsc.ru; Lotkov, Alexander I.; Ostapenko, Marina G. [Institute of Strength Physicists and Materials Science SB RAS, Tomsk, 634055 (Russian Federation); Koval, Nikolai N.; Teresov, Anton D. [National Research Tomsk State University, Tomsk, 634050 (Russian Federation); Institute of High Current Electronics SB RAS, Tomsk, 634055 (Russian Federation)

    2015-10-27

    By transmission electron microscopy method the evolution of structural-phase states on a depth of close to equiatomic NiTi modified layer has been studied. Modification performed by pulse impact on its surface low-energy high-current electron beam (beam energy density 10 J/sm{sup 2}, 10 pulses, pulse duration 50mks). It is established that during the treatment in the layer thickness of 8–10 μm, the melting of primary B2 phase and contained therein as Ti2Ni phase particles occurs. The result is change in the concentration ratio of titanium and nickel in the direction of increasing titanium content, which was confirmed by X-ray analysis in the form of increased unit cell parameter B2 phase. Analysis of the electron diffraction pattern showed that the modified layer is characterized as a highly distorted structure on the basis of bcc lattice. Lattice distortions are maximal near the surface and extends to a depth of melt. In subjacent layer there is gradual decline lattice distortions is observed.

  14. WC/Co composite surface structure and nano graphite precipitate induced by high current pulsed electron beam irradiation

    Science.gov (United States)

    Hao, S. Z.; Zhang, Y.; Xu, Y.; Gey, N.; Grosdidier, T.; Dong, C.

    2013-11-01

    High current pulsed electron beam (HCPEB) irradiation was conducted on a WC-6% Co hard alloy with accelerating voltage of 27 kV and pulse duration of 2.5 μs. The surface phase structure was examined by using glancing-angle X-ray diffraction (GAXRD), scanning electron microscope (SEM) and high resolution transmission electron microscope (HRTEM) methods. The surface tribological properties were measured. It was found that after 20 pulses of HCPEB irradiation, the surface structure of WC/Co hard alloy was modified dramatically and composed of a mixture of nano-grained WC1-x, Co3W9C4, Co3W3C phases and graphite precipitate domains ˜50 nm. The friction coefficient of modified surface decreased to ˜0.38 from 0.6 of the initial state, and the wear rate reduced from 8.4 × 10-5 mm3/min to 6.3 × 10-6 mm3/min, showing a significant self-lubricating effect.

  15. WC/Co composite surface structure and nano graphite precipitate induced by high current pulsed electron beam irradiation

    Energy Technology Data Exchange (ETDEWEB)

    Hao, S.Z., E-mail: ebeam@dlut.edu.cn [Key Laboratory of Materials Modification and School of Physics and Optoelectronics Engineering, Dalian University of Technology, Dalian 116024 (China); Zhang, Y. [Key Laboratory of Materials Modification and School of Physics and Optoelectronics Engineering, Dalian University of Technology, Dalian 116024 (China); School of Materials Science and Engineering, Shenyang University of Technology, Shenyang 110870 (China); Xu, Y. [Key Laboratory of Materials Modification and School of Physics and Optoelectronics Engineering, Dalian University of Technology, Dalian 116024 (China); College of Materials Science and Engineering, Liaoning Technical University, Fuxin 123000 (China); Gey, N.; Grosdidier, T. [Université de Lorraine, Laboratoire d’Etude des Microstructures et de Mécanique des Matériaux (LEM3), CNRS UMR 7239, Ile du Saulcy, 57045 Metz (France); Université de Lorraine, Laboratoire d’Excellence on Design of Alloy Metals for Low-Mass Structure (DAMAS), Ile du Saulcy, 57045 Metz (France); Dong, C. [Key Laboratory of Materials Modification and School of Physics and Optoelectronics Engineering, Dalian University of Technology, Dalian 116024 (China); Université de Lorraine, Laboratoire d’Excellence on Design of Alloy Metals for Low-Mass Structure (DAMAS), Ile du Saulcy, 57045 Metz (France)

    2013-11-15

    High current pulsed electron beam (HCPEB) irradiation was conducted on a WC-6% Co hard alloy with accelerating voltage of 27 kV and pulse duration of 2.5 μs. The surface phase structure was examined by using glancing-angle X-ray diffraction (GAXRD), scanning electron microscope (SEM) and high resolution transmission electron microscope (HRTEM) methods. The surface tribological properties were measured. It was found that after 20 pulses of HCPEB irradiation, the surface structure of WC/Co hard alloy was modified dramatically and composed of a mixture of nano-grained WC{sub 1−x}, Co{sub 3}W{sub 9}C{sub 4}, Co{sub 3}W{sub 3}C phases and graphite precipitate domains ∼50 nm. The friction coefficient of modified surface decreased to ∼0.38 from 0.6 of the initial state, and the wear rate reduced from 8.4 × 10{sup −5} mm{sup 3}/min to 6.3 × 10{sup −6} mm{sup 3}/min, showing a significant self-lubricating effect.

  16. Repetitively pulsed UV radiation source based on a run-away electron preionised diffuse discharge in nitrogen

    Energy Technology Data Exchange (ETDEWEB)

    Baksht, E Kh; Burachenko, A G; Lomaev, M I; Panchenko, A N; Tarasenko, V F [Institute of High Current Electronics, Siberian Branch, Russian Academy of Sciences, Tomsk (Russian Federation)

    2015-04-30

    An extended repetitively pulsed source of spontaneous UV radiation is fabricated, which may also be used for producing laser radiation. Voltage pulses with an incident wave amplitude of up to 30 kV, a half-amplitude duration of ∼4 ns and a rise time of ∼2.5 ns are applied to a gap with a nonuniform electric field. For an excitation region length of 35 cm and a nitrogen pressure of 30 – 760 Torr, a diffusive discharge up to a pulse repetition rate of 2 kHz is produced without using an additional system for gap preionisation. An investigation is made of the plasma of the run-away electron preionised diffuse discharge. Using a CCD camera it is found that the dense diffused plasma fills the gap in a time shorter than 1 ns. X-ray radiation is recorded from behind the foil anode throughout the pressure range under study; a supershort avalanche electron beam is recorded by the collector electrode at pressures below 100 Torr. (laser applications and other topics in quantum electronics)

  17. Solid state Ka-band pulse oscillator with frequency electronic switching

    Directory of Open Access Journals (Sweden)

    Dvornichenko V. P.

    2015-08-01

    Full Text Available Transmitting devices for small radars in the millimeter wavelength range with high resolution on range and noise immunity. The work presents the results of research and development of compact pulse oscillators with digital frequency switching from pulse to pulse. The oscillator consists of a frequency synthesizer and a synchronized amplifier on the IMPATT diode. Reference oscillator of synthesizer is synchronized by crystal oscillator with digital PLL system and contains a frequency multiplier and an amplifier operating in pulse mode. Small-sized frequency synthesizer of 8 mm wave lengths provides an output power of ~1.2 W per pulse with a frequency stability of no worse than 2•10–6. Radiation frequency is controlled by three-digit binary code in OOL levels. Synchronized amplifier made on IMPATT diodes provides microwave power up to 20 W in oscillator output with microwave pulse duration of 100—300 ns in an operating band. The oscillator can be used as a driving source for the synchronization of semiconductor and electro-vacuum devices of pulsed mode, and also as a transmitting device for small-sized radar of millimeter wave range.

  18. Time-dependent density-functional theory simulation for electron-ion dynamics in molecules under intense laser pulses.

    Science.gov (United States)

    Kawashita, Y; Nakatsukasa, T; Yabana, K

    2009-02-11

    We have developed a simulation method to describe three-dimensional dynamics of electrons and ions in a molecule based on the time-dependent density-functional theory. We solve the time-dependent Kohn-Sham equation for electrons employing the real-space and real-time method, while the ion dynamics are described in classical mechanics by the Ehrenfest method. For an efficient calculation in massively parallel computers, the code is parallelized dividing the spatial grid points. We apply the method to the Coulomb explosion of the H(2)S molecule under an intense and ultrashort laser pulse and investigate the mechanism of the process.

  19. New design of the pulsed electro-acoustic upper electrode for space charge measurements during electronic irradiation

    Energy Technology Data Exchange (ETDEWEB)

    Riffaud, J.; Griseri, V.; Berquez, L. [UPS, LAPLACE, Université de Toulouse, 118 Route de Narbonne, Toulouse F-31062, France and CNRS, LAPLACE, Toulouse F-31062 (France)

    2016-07-15

    The behaviour of space charges injected in irradiated dielectrics has been studied for many years for space industry applications. In our case, the pulsed electro-acoustic method is chosen in order to determine the spatial distribution of injected electrons. The feasibility of a ring-shaped electrode which will allow the measurements during irradiation is presented. In this paper, a computer simulation is made in order to determine the parameters to design the electrode and find its position above the sample. The obtained experimental results on polyethylene naphthalate samples realized during electronic irradiation and through relaxation under vacuum will be presented and discussed.

  20. New design of the pulsed electro-acoustic upper electrode for space charge measurements during electronic irradiation.

    Science.gov (United States)

    Riffaud, J; Griseri, V; Berquez, L

    2016-07-01

    The behaviour of space charges injected in irradiated dielectrics has been studied for many years for space industry applications. In our case, the pulsed electro-acoustic method is chosen in order to determine the spatial distribution of injected electrons. The feasibility of a ring-shaped electrode which will allow the measurements during irradiation is presented. In this paper, a computer simulation is made in order to determine the parameters to design the electrode and find its position above the sample. The obtained experimental results on polyethylene naphthalate samples realized during electronic irradiation and through relaxation under vacuum will be presented and discussed.

  1. Decoupling Electronic versus Nuclear Photoresponse of Isolated Green Fluorescent Protein Chromophores Using Short Laser Pulses

    Science.gov (United States)

    Kiefer, Hjalte V.; Pedersen, Henrik B.; Bochenkova, Anastasia V.; Andersen, Lars H.

    2016-12-01

    The photophysics of a deprotonated model chromophore for the green fluorescent protein is studied by femtosecond laser pulses in an electrostatic ion-storage ring. The laser-pulse duration is much shorter than the time for internal conversion, and, hence, contributions from sequential multiphoton absorption, typically encountered with ns-laser pulses, are avoided. Following single-photon excitation, the action-absorption maximum is shown to be shifted within the S0 to S1 band from its origin at about 490 to 450 nm, which is explained by the different photophysics involved in the detected action.

  2. Phase characterization of the reflection on an extreme UV multilayer: comparison between attosecond metrology and standing wave measurements

    NARCIS (Netherlands)

    Loch, R. A.; Dubrouil, A.; Sobierajski, R.; Descamps, D.; Fabre, B.; Lidon, P.; van de Kruijs, R. W. E.; Boekhout, F.; Gullikson, E.; Gaudin, J.; E. Louis,; F. Bijkerk,; Mevel, E.; Petit, S.; Constant, E.; Mairesse, Y.

    2011-01-01

    We characterize the phase shift induced by reflection on a multilayer mirror in the extreme UV range (80-93 eV) using two techniques: one based on high order harmonic generation and attosecond metrology (reconstruction of attosecond beating by interference of two-photon transitions), and a second

  3. Hybrid insulation coordination and optimisation for 1 MV operation of pulsed electron accelerator KALI-30GW

    Energy Technology Data Exchange (ETDEWEB)

    Senthil, K.; Mitra, S.; Sandeep, S., E-mail: sentilk@barc.gov.in [Accelerator and Pulse Power Division, Bhabha Atomic Research Centre, Mumbai (India); and others

    2014-07-01

    In a multi-gigawatt pulsed power system like KALI-30 GW, insulation coordination is required to achieve high voltages ranging from 0.3 MV to 1 MV. At the same time optimisation of the insulation parameters is required to minimize the inductance of the system, so that nanoseconds output can be achieved. The KALI-30GW pulse power system utilizes a combination of Perspex, delrin, epoxy, transformer oil, nitrogen/SF{sub 6} gas and vacuum insulation at its various stages in compressing DC high voltage to a nanoseconds pulse. This paper describes the operation and performance of the system from 400 kV to 1030 kV output voltage pulse and insulation parameters utilized for obtaining peak 1 MV output. (author)

  4. Physical Kinetics of Electrons in a High-Voltage Pulsed High-Pressure Discharge with Cylindrical Geometry

    Science.gov (United States)

    Kozhevnikov, V. Yu.; Kozyrev, A. V.; Semeniuk, N. S.

    2017-12-01

    Results of theoretical modeling of the phenomenon of a high-voltage discharge in nitrogen at atmospheric pressure are presented, based on a consistent kinetic theory of the electrons. A mathematical model of a nonstationary high-pressure discharge has been constructed for the first time, based on a description of the electron component from first principles. The physical kinetics of the electrons are described with the help of the Boltzmann kinematic equation for the electron distribution function over momenta with only ionization and elastic collisions taken into account. A detailed spatiotemporal picture of a nonstationary discharge with runaway electrons under conditions of coaxial geometry of the gas diode is presented. The model describes in a self-consistent way both the process of formation of the runaway electron flux in the discharge and the influence of this flux on the rate of ionization processes in the gas. Total energy spectra of the electron flux incident on the anode are calculated. The obtained parameters of the current pulse of the beam of fast electrons correlate well with the known experimental data.

  5. Influence of a step-tapered undulator field on the optical pulse shape of a far-infrared free-electron laser

    NARCIS (Netherlands)

    Knippels, G.M.H.; van der Meer, A. F. G.; R F X A M Mols,; Oepts, D.; van Amersfoort, P. W.; Jaroszynski, D. A.

    1996-01-01

    The optical output of the free-electron laser for infrared experiments (FELIX), which operates in the regime of strong slippage, consists of picosecond pulses, Depending on the amount of cavity desynchronization, the optical pulse can develop substantial structure in the form of multiple subpulses,

  6. Capturing atomic-scale carrier dynamics with electrons

    Science.gov (United States)

    Baum, Peter; Krausz, Ferenc

    2017-09-01

    Light-driven electronic motion unfolds on times as short as the cycle period of light and on length scales as small as the distance between two neighboring atoms in a molecule. Visualizing fundamental light-matter interactions therefore requires access to attosecond and picometer dimensions. Here we report on a potential unification of electron diffraction and microscopy with attosecond technology, which could provide a full space-time access to elementary electronic processes in matter and materials. We review recent progress in ultrafast diffraction and microscopy towards temporal resolutions approaching 10 fs by use of state-of-the-art microwave technology and discuss our latest findings on all-optical compression approaches for reaching sub-femtosecond, sub-optical-cycle resolution. Four-dimensional electron diffraction with attosecond-picometer resolution will access all dynamics outside the atomic core, offering an all-embracing insight into fundamental electron-nuclear dynamics of complex materials.

  7. Repetitively pulsed UV radiation source based on a run-away electron preionised diffuse discharge in nitrogen

    Science.gov (United States)

    Baksht, E. Kh; Burachenko, A. G.; Lomaev, M. I.; Panchenko, A. N.; Tarasenko, V. F.

    2015-04-01

    An extended repetitively pulsed source of spontaneous UV radiation is fabricated, which may also be used for producing laser radiation. Voltage pulses with an incident wave amplitude of up to 30 kV, a half-amplitude duration of ~4 ns and a rise time of ~2.5 ns are applied to a gap with a nonuniform electric field. For an excitation region length of 35 cm and a nitrogen pressure of 30 - 760 Torr, a diffusive discharge up to a pulse repetition rate of 2 kHz is produced without using an additional system for gap preionisation. An investigation is made of the plasma of the run-away electron preionised diffuse discharge. Using a CCD camera it is found that the dense diffused plasma fills the gap in a time shorter than 1 ns. X-ray radiation is recorded from behind the foil anode throughout the pressure range under study; a supershort avalanche electron beam is recorded by the collector electrode at pressures below 100 Torr.

  8. Electron slicing for the generation of tunable femtosecond soft x-ray pulses from a free electron laser and slice diagnostics

    Directory of Open Access Journals (Sweden)

    S. Di Mitri

    2013-04-01

    Full Text Available We present the experimental results of femtosecond slicing an ultrarelativistic, high brightness electron beam with a collimator. In contrast to some qualitative considerations reported in Phys. Rev. Lett. 92, 074801 (2004PRLTAO0031-900710.1103/PhysRevLett.92.074801, we first demonstrate that the collimation process preserves the slice beam quality, in agreement with our theoretical expectations, and that the collimation is compatible with the operation of a linear accelerator in terms of beam transport, radiation dose, and collimator heating. Accordingly, the collimated beam can be used for the generation of stable femtosecond soft x-ray pulses of tunable duration, from either a self-amplified spontaneous emission or an externally seeded free electron laser. The proposed method also turns out to be a more compact and cheaper solution for electron slice diagnostics than the commonly used radio frequency deflecting cavities and has minimal impact on the machine design.

  9. Laser-assisted electron scattering in strong-field ionization of dense water vapor by ultrashort laser pulses

    Science.gov (United States)

    Wilke, M.; Al-Obaidi, R.; Moguilevski, A.; Kothe, A.; Engel, N.; Metje, J.; Kiyan, I. Yu; Aziz, E. F.

    2014-08-01

    We report on strong-field ionization of dense water gas in a short infrared laser pulse. By employing a unique combination of photoelectron spectroscopy with a liquid micro-jet technique, we observe how the character of electron emission at high kinetic energies changes with the increase of the medium density. This change is associated with the process of laser-assisted electron scattering (LAES) on neighboring particles, which becomes a dominant mechanism of hot electron emission at higher medium densities. The manifestation of this mechanism is found to require densities that are orders of magnitude lower than those considered for heating the laser-generated plasmas via the LAES process. The experimental results are supported by simulations of the LAES yield with the use of the Kroll-Watson theory.

  10. Very low electron temperature in warm dense matter formed by focused picosecond soft x-ray laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Ishino, Masahiko, E-mail: ishino.masahiko@jaea.go.jp; Hasegawa, Noboru; Nishikino, Masaharu; Kawachi, Tetsuya; Yamagiwa, Mitsuru [Quantum Beam Science Center, Japan Atomic Energy Agency, 8-1-7, Umemidai, Kizugawa, Kyoto 619-0215 (Japan); Pikuz, Tatiana [Joint Institute for High Temperatures, Russian Academy of Sciences, 13-2, Izhorskaya Street, Moscow 125412 (Russian Federation); Graduate School of Engineering, Osaka University, 1-1, Yamadaoka, Suita, Osaka 565-0871 (Japan); Skobelev, Igor [Joint Institute for High Temperatures, Russian Academy of Sciences, 13-2, Izhorskaya Street, Moscow 125412 (Russian Federation); National Research Nuclear University, Moscow Engineering Physics Institute, 31, Kashirskoe Shosse, Moscow 115409 (Russian Federation); Faenov, Anatoly [Joint Institute for High Temperatures, Russian Academy of Sciences, 13-2, Izhorskaya Street, Moscow 125412 (Russian Federation); Institute for Academic Initiatives, Osaka University, 1-1, Yamadaoka, Suita, Osaka 565-0871 (Japan); Inogamov, Nail [Landau Institute for Theoretical Physics, Russian Academy of Sciences, 1-A, Akademika Semenova av., Chernogolovka, Moscow Region 142432 (Russian Federation)

    2014-11-14

    We investigated the optical emission from the ablating surfaces induced by the irradiations of soft x-ray laser (SXRL) pulses with the aim of estimation of the maximum electron temperature. No emission signal in the spectral range of 400–800 nm could be observed despite the formation of damage structures on the target surfaces. Hence, we estimated an upper limit for the electron temperature of 0.4–0.7 eV for the process duration of 100–1000 ps. Our results imply that the ablation and/or surface modification by the SXRL is not accompanied by plasma formation but is induced by thermo-mechanical pressure, which is so called a spallative ablation. This spallative ablation process occurs in the low electron temperature region of a non-equilibrium state of warm dense matter.

  11. Optical features of a LiF crystal soft X-ray imaging detector irradiated by free electron laser pulses.

    Science.gov (United States)

    Pikuz, Tatiana; Faenov, Anatoly; Fukuda, Yuji; Kando, Masaki; Bolton, Paul; Mitrofanov, Alexander; Vinogradov, Alexander; Nagasono, Mitsuru; Ohashi, Haruhiko; Yabashi, Makina; Tono, Kensuke; Senba, Yashinori; Togashi, Tadashi; Ishikawa, Tetsuya

    2012-02-13

    Optical features of point defects photoluminescence in LiF crystals, irradiated by soft X-ray pulses of the Free Electron Laser with wavelengths of 17.2 - 61.5 nm, were measured. We found that peak of photoluminescence spectra lies near of 530 nm and are associated with emission of F3+ centers. Our results suggest that redistribution of photoluminescence peak intensity from the red to the green part of the spectra is associated with a shortening of the applied laser pulses down to pico - or femtosecond durations. Dependence of peak intensity of photoluminescence spectra from the soft X-ray irradiation fluence was measured and the absence of quenching phenomena, even at relatively high fluencies was found, which is very important for wide applications of LiF crystal X-ray imaging detectors.

  12. Effect of pulsed voltage on electrochemical migration of tin in electronics

    DEFF Research Database (Denmark)

    Verdingovas, Vadimas; Jellesen, Morten Stendahl; Ambat, Rajan

    2015-01-01

    respectively at 10 and 5 V, while the duty cycle and the pulse width were varied in the range of ms. The results showed that varying of pulse width at fixed duty cycle has a minor effect under investigated conditions, whereas increasing duty cycle significantly reduces the time to short due to dendrite...... formation and increases the charge transferred between the electrodes over time. With increase of duty cycle, increases the anodic dissolution of tin, which was visualized using a tin ion indicator applied on the components prior to applying the voltage. The anodic dissolution of tin significantly...... influences the dendritic growth, although a tendency for more hydroxide precipitation was observed for lower duty cycles. The precipitation of tin hydroxides was identified as influencing factor for the reduction of charge transfer under pulsed voltage with low duty cycles, therefore resulting...

  13. The electromagnetic radiation fields of a relativistic electron avalanche with special attention to the origin of narrow bipolar pulses

    Science.gov (United States)

    Cooray, G. V.; Cooray, G. K.

    2011-12-01

    Gurevich et al. [1] postulated that the source of narrow bipolar pulses, a class of high energy pulses that occur during thunderstorms, could be a runaway electron avalanche driven by the intense electric fields of a thunderstorm. Recently, Watson and Marshall [2] used the modified transmission line model to test the mechanism of the source of narrow bipolar pulses. In a recent paper, Cooray and Cooray [3] demonstrated that the electromagnetic fields of accelerating charges could be used to evaluate the electromagnetic fields from electrical discharges if the temporal and spatial variation of the charges in the discharge is known. In the present study, those equations were utilized to evaluate the electromagnetic fields generated by a relativistic electron avalanche. In the analysis it is assumed that all the electrons in the avalanche are moving with the same speed. In other words, the growth or the decay of the number of electrons takes place only at the head of the avalanche. It is shown that the radiation is emanating only from the head of the avalanche where electrons are being accelerated. It is also shown that an analytical expression for the radiation field of the avalanche at any distance can be written directly in terms of the e-folding length of the avalanche. This makes it possible to extract directly the spatial variation of the e-folding length of the avalanche from the measured radiation fields. In the study this model avalanche was used to investigate whether it can be used to describe the measured electromagnetic fields of narrow bipolar pulses. The results obtained are in reasonable agreement with the two station data of Eack [4] for speeds of propagation around (2 - 2.5) x 10^8 m/s and when the propagation effects on the electric fields measured at the distant station is taken into account. [1] Gurevich et al. (2004), Phys. Lett. A., 329, pp. 348 -361. [2] Watson, S. S. and T. C. Marshall (2007), Geophys. Res. Lett., Vol. 34, L04816, doi: 10

  14. Design and implementation of an optimal laser pulse front tilting scheme for ultrafast electron diffraction in reflection geometry with high temporal resolution

    Directory of Open Access Journals (Sweden)

    Francesco Pennacchio

    2017-07-01

    Full Text Available Ultrafast electron diffraction is a powerful technique to investigate out-of-equilibrium atomic dynamics in solids with high temporal resolution. When diffraction is performed in reflection geometry, the main limitation is the mismatch in group velocity between the overlapping pump light and the electron probe pulses, which affects the overall temporal resolution of the experiment. A solution already available in the literature involved pulse front tilt of the pump beam at the sample, providing a sub-picosecond time resolution. However, in the reported optical scheme, the tilted pulse is characterized by a temporal chirp of about 1 ps at 1 mm away from the centre of the beam, which limits the investigation of surface dynamics in large crystals. In this paper, we propose an optimal tilting scheme designed for a radio-frequency-compressed ultrafast electron diffraction setup working in reflection geometry with 30 keV electron pulses containing up to 105 electrons/pulse. To characterize our scheme, we performed optical cross-correlation measurements, obtaining an average temporal width of the tilted pulse lower than 250 fs. The calibration of the electron-laser temporal overlap was obtained by monitoring the spatial profile of the electron beam when interacting with the plasma optically induced at the apex of a copper needle (plasma lensing effect. Finally, we report the first time-resolved results obtained on graphite, where the electron-phonon coupling dynamics is observed, showing an overall temporal resolution in the sub-500 fs regime. The successful implementation of this configuration opens the way to directly probe structural dynamics of low-dimensional systems in the sub-picosecond regime, with pulsed electrons.

  15. Interaction of short x-ray pulses with low-Z x-ray optics materials at the LCLS free-electron laser.

    Science.gov (United States)

    Hau-Riege, S P; London, R A; Graf, A; Baker, S L; Soufli, R; Sobierajski, R; Burian, T; Chalupsky, J; Juha, L; Gaudin, J; Krzywinski, J; Moeller, S; Messerschmidt, M; Bozek, J; Bostedt, C

    2010-11-08

    Materials used for hard x-ray-free-electron laser (XFEL) optics must withstand high-intensity x-ray pulses. The advent of the Linac Coherent Light Source has enabled us to expose candidate optical materials, such as bulk B4C and SiC films, to 0.83 keV XFEL pulses with pulse energies between 1 μJ and 2 mJ to determine short-pulse hard x-ray damage thresholds. The fluence required for the onset of damage for single pulses is around the melt fluence and slightly lower for multiple pulses. We observed strong mechanical cracking in the materials, which may be due to the larger penetration depths of the hard x-rays.

  16. Surface nanostructure and improved microhardness of 40CrNiMo7 steel induced by high current pulsed electron beam treatment

    Science.gov (United States)

    Wang, Huihui; Hao, Shengzhi

    2017-07-01

    In this paper, surface modification of 40CrNiMo7 steel was investigated with high current pulsed electron beam (HCPEB) treatment. The scanning electron microscope (SEM), electron back-scattered diffraction (EBSD), electron probe micro analysis (EPMA), transmission electron microscopy (TEM) and X-ray diffraction (XRD) results show that a composite microstructure of mainly refined austenite and a little martensite was produced in the surface modified layer of depth ∼7 μm. The average size of small cells on modified surface was decreased to ∼120 nm after 25 HCPEB pulses. XRD analysis indicates a preferred orientation of austenite (2 2 0) crystal plane, and TEM results show the broken and dissolved cementite in the surface modified layer. After HCPEB treatment, all the samples exhibited a remarkable improvement in surface microhardness measurement, up to ∼1000 HK for 15 HCPEB pulses, as tripled of the initial 40CrNiMo7 steel.

  17. Nanostructure Formations and Improvement in Corrosion Resistance of Steels by Means of Pulsed Electron Beam Surface Treatment

    Directory of Open Access Journals (Sweden)

    K. M. Zhang

    2013-01-01

    Full Text Available The corrosion of steels has long been the topic for materials scientists. It is established that surface treatment is an efficient way to improve the corrosion resistance of steels without changing the bulk properties and with low costs. In the present paper, different kinds of surface treatment techniques for steels are briefly reviewed. In particular, the surface modification involving nanostructure formations of steels by using a low energy high pulsed electron beam (LEHCPEB treatment is lightened in the case of an AISI 316L stainless steel and D2 steel. The overall results demonstrate the high potential of the LEHCPEB technique for improving the corrosion performance of steels.

  18. Theoretical and experimental study of superradiance pulse generation by heavy-current subnanosecond electron bunches moving in periodic slowing down system

    CERN Document Server

    Ginzburg, N S; Novozhilova, Y V; Sergeev, A S; Shpak, V G; Shunailov, S A; Ul'maskulov, M R; Yalandin, M I

    2002-01-01

    One studied both theoretically and experimentally the Cherenkov superradiance at liner motion of an electron bunch through the periodic slowing down system. Simulations in terms of the KARAT code show that peak intensity of microwave pulses is proportional to the square of total number of particles in a bunch. This finding os conformed experimentally. As a results, at 39 GHz frequency one obtained ultrashort pulses of up to 140 MW high intensity and with 30 ps duration. The RADAN 303 high-current subnanosecond accelerator injected electron bunches with up to 2 A current, 0.5-1.5 ns duration and 200-300 keV particle energy was used as a source of electrons. Simulation shows possibility of further intensification of electromagnetic pulses up to 300-400 MW due to optimization of parameters of accelerating voltage pulse

  19. Comparative study of amplified spontaneous emission and short pre-pulse impacts onto fast electron generation at sub-relativistic femtosecond laser-plasma interaction

    Science.gov (United States)

    Ivanov, K. A.; Shulyapov, S. A.; Ksenofontov, P. A.; Tsymbalov, I. N.; Volkov, R. V.; Savel'ev, A. B.; Brantov, A. V.; Bychenkov, V. Yu.; Turinge, A. A.; Lapik, A. M.; Rusakov, A. V.; Djilkibaev, R. M.; Nedorezov, V. G.

    2014-09-01

    This paper describes the study of hot electron generation under the action of intense (˜1018 W/cm2) femtosecond pulses onto the surface of a solid target, in the presence of a long pre-plasma, which varied with different spatial extents and densities. The corona was formed by pre-pulses with varied intensities and temporal profiles (amplified spontaneous emission (ASE) and short pre-pulses). The most efficient fast electron acceleration, to energies well beyond the ponderomotive potential, was observed if the ASE was able to form to the extent of ˜100 μm a slightly undercritical plasma. Energy of accelerated electrons underwent further growth if the laser pulse duration increased from ˜45 to ˜350 fs at constant energy fluence. The experimental results were supported by numerical simulations using 3D3V Mandor PIC code.

  20. Electron-ion coupling and ambipolar diffusion in dense electron-hole plasma in thin amorphous Si films studied by single-shot, pulse-width dependent ultrafast laser ablation

    Science.gov (United States)

    Danilov, Pavel; Ionin, Andrey; Khmelnitskii, Roman; Kiseleva, Irina; Kudryashov, Sergey; Mel'nik, Nikolay; Rudenko, Andrey; Smirnov, Nikita; Zayarny, Dmitry

    2017-12-01

    Single-shot ablation of amorphous silicon films of 50-, 100- and 150-nm thickness by laser pulses of variable (0.2-6 ps) widths demonstrates non-monotonous variation of ablation thresholds and characteristic ablation 1/e-radii with their minima at the 0.6-ps pulse-width and the following increase. For the shorter laser pulses the increased thresholds and enhanced transport can be related to fast ambipolar electron-hole plasma diffusion and other electronic energy losses in dense transient plasma prior its energy transfer to the ionic subsystem (electron-ion thermalization) at 0.6 ps, while for the longer laser pulses slower ambipolar diffusion in moderate-density electron-hole plasma, ionic heat conduction and other thermal losses may predominate.

  1. Damage effect and mechanism of the GaAs pseudomorphic high electron mobility transistor induced by the electromagnetic pulse

    Science.gov (United States)

    Xiao-Wen, Xi; Chang-Chun, Chai; Gang, Zhao; Yin-Tang, Yang; Xin-Hai, Yu; Yang, Liu

    2016-04-01

    The damage effect and mechanism of the electromagnetic pulse (EMP) on the GaAs pseudomorphic high electron mobility transistor (PHEMT) are investigated in this paper. By using the device simulation software, the distributions and variations of the electric field, the current density and the temperature are analyzed. The simulation results show that there are three physical effects, i.e., the forward-biased effect of the gate Schottky junction, the avalanche breakdown, and the thermal breakdown of the barrier layer, which influence the device current in the damage process. It is found that the damage position of the device changes with the amplitude of the step voltage pulse. The damage appears under the gate near the drain when the amplitude of the pulse is low, and it also occurs under the gate near the source when the amplitude is sufficiently high, which is consistent with the experimental results. Project supported by the National Basic Research Program of China (Grant No. 2014CB339900), and the Open Fund of Key Laboratory of Complex Electromagnetic Environment Science and Technology, China Academy of Engineering Physics (CAEP) (Grant No. 2015-0214.XY.K).

  2. Luminescence induced by electrons outside zinc oxide nanoparticles driven by intense terahertz pulse trains

    Science.gov (United States)

    Nagai, Masaya; Aono, Shingo; Ashida, Masaaki; Kawase, Keigo; Irizawa, Akinori; Isoyama, Goro

    2017-05-01

    We investigated the behaviours of electrons from ZnO nanoparticles via a strong terahertz field. Luminescence from ZnO nanoparticles and surrounding nitrogen molecules was observed when the nanoparticles were irradiated with a terahertz free-electron laser (FEL). These excitations arose from the collision of electrons released via field electron emission with the ZnO nanoparticles and neighbouring nitrogen molecules. The strong excitation frequency dependence of the luminescence reflected the kinetic energy and trajectory of electrons outside the nanoparticles. We also observed spectral changes in the luminescence during macropulses of the FEL, even though the carrier lifetime of the nanoparticles was shorter than the interval between the micropulses. These changes were caused by the nanoparticles becoming charged due to electron emission, resulting in the electrons being re-emitted outside the nanoparticles. The electrons outside the nanoparticles were accelerated more efficiently by the terahertz field than the electrons inside the nanoparticles, and thus the motion of these exterior electrons provided a new excitation path.

  3. Quantum switching of π-electron rotations in a nonplanar chiral molecule by using linearly polarized UV laser pulses.

    Science.gov (United States)

    Mineo, Hirobumi; Yamaki, Masahiro; Teranishi, Yoshiaki; Hayashi, Michitoshi; Lin, Sheng Hsien; Fujimura, Yuichi

    2012-09-05

    Nonplanar chiral aromatic molecules are candidates for use as building blocks of multidimensional switching devices because the π electrons can generate ring currents with a variety of directions. We employed (P)-2,2'-biphenol because four patterns of π-electron rotations along the two phenol rings are possible and theoretically determine how quantum switching of the π-electron rotations can be realized. We found that each rotational pattern can be driven by a coherent excitation of two electronic states under two conditions: one is the symmetry of the electronic states and the other is their relative phase. On the basis of the results of quantum dynamics simulations, we propose a quantum control method for sequential switching among the four rotational patterns that can be performed by using ultrashort overlapped pump and dump pulses with properly selected relative phases and photon polarization directions. The results serve as a theoretical basis for the design of confined ultrafast switching of ring currents of nonplanar molecules and further current-induced magnetic fluxes of more sophisticated systems.

  4. Surface Nanocrystallization of 3Cr13 Stainless Steel Induced by High-Current Pulsed Electron Beam Irradiation

    Directory of Open Access Journals (Sweden)

    Zhiyong Han

    2013-01-01

    Full Text Available The nanocrystalline surface was produced on 3Cr13 martensite stainless steel surface using high-current pulsed electron beam (HCPEB technique. The structures of the nanocrystallized surface were characterized by X-ray diffraction and electron microscopy. Two nanostructures consisting of fine austenite grains (50–150 nm and very fine carbides precipitates are formed in melted surface layer after multiple bombardments via dissolution of carbides and crater eruption. It is demonstrated that the dissolution of the carbides and the formation of the supersaturated Fe (C solid solution play a determining role on the microstructure evolution. Additionally, the formation of fine austenite structure is closely related to the thermal stresses induced by the HCPEB irradiation. The effects of both high carbon content and high value of stresses increase the stability of the austenite, which leads to the complete suppression of martensitic transformation.

  5. Design principles for high quality electron beams via colliding pulses in laser plasma accelerators

    Directory of Open Access Journals (Sweden)

    E. Cormier-Michel

    2014-09-01

    Full Text Available Laser plasma based accelerators have the potential to reduce dramatically the size and cost of future particle colliders and light sources. Production of high quality beams along with reproducibility, tunability, and efficiency are required for many applications. We present design principles for two-pulse colliding laser pulse injection mechanisms, which can meet these requirements. Simulations are used to determine the best conditions for the production of high quality beams: high charge, low energy spread, and low emittance. Simulations also allow access to the internal dynamics of the interaction, providing insight regarding further improvement of the beam quality. We find that a 20 pC beam can be accelerated to 300 MeV in 4 mm with only a few percent energy spread and transverse normalized emittance close to 1 mm mrad, using a 10 TW laser. We demonstrate that this design scales according to linear theory. Control of the laser pulse mode content and subsequent evolution in the plasma channel are shown to be critical for achieving the highest beam quality.

  6. Measurements of the temporal and spatial phase variations of a 33 GHz pulsed free electron laser amplifier and application to high gradient RF acceleration

    Energy Technology Data Exchange (ETDEWEB)

    Volfbeyn, P.; Bekefi, G. [Massachusetts Institute of Technology, Cambridge, MA (United States)

    1995-12-31

    We report the results of temporal and spatial measurements of phase of a pulsed free electron laser amplifier (FEL) operating in combined wiggler and axial guide magnetic fields. The 33 GHz FEL is driven by a mildly relativistic electron beam (750 kV, 90-300 A, 30 ns) and generates 61 MW of radiation with a high power magnetron as the input source. The phase is measured by an interferometric technique from which frequency shifting is determined. The results are simulated with a computer code. Experimental studies on a CERN-CLIC 32.98 GHz 26-cell high gradient accelerating section (HGA) were carried out for input powers from 0.1 MW to 35 MW. The FEL served as the r.f. power source for the HGA. The maximum power in the transmitted pulse was measured to be 15 MW for an input pulse of 35 MW. The theoretically calculated shunt impedance of 116 M{Omega}/m predicts a field gradient of 65 MeV/m inside the HGA. For power levels >3MW the pulse transmitted through the HGA was observed to be shorter than the input pulse and pulse shortening became more serious with increasing power input. At the highest power levels the output pulse length (about 5 nsec) was about one quarter of the input pulse length. Various tests suggest that these undesirable effects occur in the input coupler to the HGA. Light and X-ray production inside the HGA have been observed.

  7. Slippage effect on energy modulation in seeded free-electron lasers with frequency chirped seed laser pulses

    Directory of Open Access Journals (Sweden)

    Chao Feng

    2013-06-01

    Full Text Available Free-electron lasers (FELs seeded with external lasers hold great promise for generating high power radiation with nearly transform-limited bandwidth in the soft x-ray region. However, it has been pointed out that the initial seed laser phase error will be amplified by the frequency up-conversion process, which may degrade the quality of the output radiation produced by a harmonic generation scheme. In this paper, theoretical and simulation studies on frequency chirp amplification in seeded FEL schemes with slippage effect taken into account are presented. It is found that the seed laser imperfection experienced by the electron beam can be significantly smoothed by the slippage effect in the modulator when the slippage length is comparable to the seed laser pulse length. This smoothing effect allows one to preserve the excellent temporal coherence of seeded FELs in the presence of large frequency chirp in the seed laser. Our studies show that the tolerance on frequency chirp in the seed laser for generating nearly transform-limited soft x-ray pulses in seeded FELs is much looser than previously thought and fully coherent radiation at nanometer wavelength may be reached with current technologies.

  8. Strengthening effect of nano-scaled precipitates in Ta alloying layer induced by high current pulsed electron beam

    Energy Technology Data Exchange (ETDEWEB)

    Tang, Guangze; Luo, Dian; Fan, Guohua [School of Material Science & Engineering, Harbin Institute of Technology, Harbin 150001 (China); Ma, Xinxin, E-mail: maxin@hit.edu.cn [State Key Laboratory of Advanced Welding and Joining, Harbin Institute of Technology, Harbin 150001 (China); Wang, Liqin [School of Mechatronics Engineering, Harbin Institute of Technology, Harbin 150001 (China)

    2017-05-01

    Highlights: • Ta alloying layer are fabricated by magnetron sputtering and high current pulsed electron beam. • Nano-scaled TaC precipitates forms within the δ-Fe grain after tempering treatment. • The mean diameter of TaC particles is about 5–8 nm. • The hardness of alloying layer increased by over 50% after formation of nano-scaled TaC particle. - Abstract: In this study, the combination of magnetron sputtering and high current pulsed electron beam are used for surface alloying treatment of Ta film on high speed steel. And the Ta alloying layer is about 6 μm. After tempering treatment, TaC phase forms in Ta alloying layer when the treated temperature is over 823 K. Through the TEM and HRTEM observation, a large amount of nano-scaled precipitates (mean diameter 5–8 nm) form within the δ-Fe grain in Ta alloying layer after tempering treatment and these nano-scaled precipitates are confirmed as TaC particles, which contribute to the strengthening effect of the surface alloying layer. The hardness of tempered alloying layer can reach to 18.1 GPa when the treated temperature is 823 K which increase by 50% comparing with the untreated steel sample before surface alloying treatment.

  9. Quantum coherent π-electron rotations in a non-planar chiral molecule induced by using a linearly polarized UV laser pulse

    Science.gov (United States)

    Mineo, Hirobumi; Fujimura, Yuichi

    2015-06-01

    We propose an ultrafast quantum switching method of π-electron rotations, which are switched among four rotational patterns in a nonplanar chiral aromatic molecule (P)-2,2’- biphenol and perform the sequential switching among four rotational patterns which are performed by the overlapped pump-dump laser pulses. Coherent π-electron dynamics are generated by applying the linearly polarized UV pulse laser to create a pair of coherent quasidegenerated excited states. We also plot the time-dependent π-electron ring current, and discussed ring current transfer between two aromatic rings.

  10. Quantum Localization of Coherent π-Electron Angular Momentum in (P)-2,2'-Biphenol.

    Science.gov (United States)

    Yamaki, Masahiro; Mineo, Hirobumi; Teranishi, Yoshiaki; Hayashi, Michitoshi; Fujimura, Yuichi; Nakamura, Hiroki; Lin, Sheng Hsien

    2014-06-05

    Controlling π-electrons with delocalized character is one of the fundamental issues in femtosecond and attosecond chemistry. Localization of π-electron rotation by using laser pulses is expected to play an essential role in nanoscience. The π-electron rotation created at a selected aromatic ring of a single molecule induces a local intense electromagnetic field, which is a new type of ultrafast optical control functioning. We propose a quantum localization of coherent π-electron angular momentum in (P)-2,2'-biphenol, which is a simple, covalently linked chiral aromatic ring chain molecule. The localization considered here consists of sequential two steps: the first step is to localize the π-electron angular momentum at a selected ring of the two benzene rings, and the other is to maintain the localization. Optimal control theory was used for obtaining the optimized electric fields of linearly polarized laser pulses to realize the localization. The optimal electric fields and the resultant coherent electronic dynamics are analyzed.

  11. Desorption of H atoms from graphite (0001) using XUV free electron laser pulses

    DEFF Research Database (Denmark)

    Siemer, B.; Olsen, Thomas; Hoger, T.

    2010-01-01

    , and identifies the highest vibrational state in the adsorbate potential as a major source for the slow atoms. It is evident that multiple electron scattering processes are required for this desorption. A direct electronic excitation of a repulsive hydrogen-carbon bond seems not to be important....

  12. PFI-ZEKE (Pulsed Field Ionization-Zero Electron Kinetic Energy) para el estudio de iones

    Science.gov (United States)

    Castaño, F.; Fernández, J. A.; Basterretxea, A. Longarte. F.; Sánchez Rayo, M. N.; Martínez, R.

    Entre las áreas hacia donde ha evolucionado la Química en los últimos años están los estudios de sistemas con especies reactivas de alta energía y los dominados por fuerzas intermoleculares débiles, con energías de unas pocas kcal/mol. En efecto, el estudio de las propiedades de los iones, comenzando por su relación con la molécula neutra de la que procede, la energía de ionización, los estados vibracionales y rotacionales, energías de enlace de Van der Waals entre el ión y una amplia variedad de otras moléculas, sus confórmeros o isómeros y sus reacciones o semi-reacciones químicas están en la raíz de la necesidad de la espectroscopía conocida como PFI-ZEKE, Pulsed Field Ionization-Zero Electron Kinetic Energy. Entre las aplicaciones que requieren estos conocimientos se encuentran la generación de plasmas para la fabricación de semiconductores, memorias magnéticas, etc, así como los sistemas astrofísicos, la ionosfera terrestre, etc. La espectroscopía ZEKE es una evolución de las de fluorescencia inducida por láser, LIF, ionización multifotónica acrecentada por resonancia, REMPI, con uno y dos colores y acoplada a un sistema de tiempo de vuelo, REMPI-TOF-MS, y las espectroscopías de doble resonancia IR-UV y UV-UV. Sus espectros y la ayuda de cálculos ab inicio permite determinar las energías de enlace de complejos de van der Waals en estados fundamental y excitados, identificar confórmeros e isómeros, obtener energías de ionización experimentales aproximadas (100 cm-1) y otras variables de interés. Al igual que con LIF, REMPI y dobles resonancias, es posible utilizar muestras gaseosas, pero los espectros están muy saturados de bandas y su interpretación es difícil o imposible. Se evitan estas dificultades estudiando las moléculas o complejos en expansiones supersónicas, donde la T de los grados de libertad solo alcanzan unos pocos K. Para realizar experimentos de ZEKE hay que utilizar una propiedad recientemente

  13. Effects of Thickness, Pulse Duration, and Size of Strip Electrode on Ferroelectric Electron Emission of Lead Zirconate Titanate Films

    Science.gov (United States)

    Yaseen, Muhammad; Ren, Wei; Chen, Xiaofeng; Feng, Yujun; Shi, Peng; Wu, Xiaoqing

    2017-11-01

    Sol-gel-derived lead zirconate titanate (PZT) thin-film emitters with thickness up to 9.8 μm have been prepared on Pt/TiO2/SiO2/Si wafer via chemical solution deposition with/without polyvinylpyrrolidone (PVP) modification, and the relationship between the film thickness and electron emission investigated. Notable electron emission was observed on application of a trigger voltage of 120 V for PZT film with thickness of 1.1 μm. Increasing the film thickness decreased the threshold field to initiate electron emission for non-PVP-modified films. In contrast, the electron emission behavior of PVP-modified films did not show significant dependence on film thickness, probably due to their porous structure. The emission current increased with decreasing strip width and space between strips. Furthermore, it was observed that increasing the duration of the applied pulse increased the magnitude of the emission current. The stray field on the PZT film thickness was also calculated and found to increase with increasing ferroelectric sample thickness. The PZT emitters were found to be fatigue free up to 105 emission cycles. Saturated emission current of around 25 mA to 30 mA was achieved for the electrode pattern used in this work.

  14. Electric propulsion. [pulsed plasma thruster and electron bombardment ion engine for MSAT attitude control and stationkeeping

    Science.gov (United States)

    1982-01-01

    An alternative propulsion subsystem for MSAT is presented which has a potential of reducing the satellite weight by more than 15%. The characteristics of pulsed plasma and ion engines are described and used to estimate of the mass of the propellant and thrusters for attitude control and stationkeeping functions for MSAT. Preliminary estimates indicate that the electric propulsion systems could also replace the large momentum wheels necessary to counteract the solar pressure; however, the fine pointing wheels would be retained. Estimates also show that either electric propulsion system can save approximately 18% to 20% of the initial 4,000 kg mass. The issues that require further experimentation are mentioned.

  15. CALCULATION-EXPERIMENTAL METHOD OF RESEARCH IN A METALLIC CONDUCTOR WITH THE PULSE CURRENT OF ELECTRONIC WAVEPACKAGES AND DE BROGLIE ELECTRONIC HALF-WAVES

    Directory of Open Access Journals (Sweden)

    M. I. Baranov

    2016-12-01

    Full Text Available Purpose. Development of calculation-experimental method for a discovery and study of electronic wavepackages (EWP and of de Broglie electronic half-waves in a metallic conductor with the pulse axial-flow current of high density. Methodology. Theoretical bases of the electrical engineering, bases of quantum physics, electrophysics bases of technique of high voltage and large pulsecurrents, and also bases of technique of measuring of permanent and variable electric value. Results. On the basis of generalization of results of research of features of the longitudinal wave periodic distributing of negatively charged transmitters of electric current of conductivity in the thin round continuous zincked steel wire offered and approved in the conditions of high-voltage laboratory method for a discovery and direct determination in him of geometrical parameters of «hot» and «cold» longitudinal areas quantized periodic longitudinal EWP and accordingly the mediated determination of values of the quantized lengths formative their de Broglie electronic half-waves. It is shown that results of close quantum mechanical calculations of EWP and quantized lengths λenz/2 of longitudinal de Broglie half-waves for the probed wire long l0 well comport with the results of the executed high temperature experiments on the powerful high-voltage generator of homopolar large pulse current of millisecond duration. Originality. First calculation-experimental a way the important for the theory of electricity fact of existence is set in a round metallic explorer with the impulsive axial-flow current of the quantized coherent de Broglie electronic half-waves, amplitudes of which at the quantum number of n=1,3,9 correspond the middles of «hot» longitudinal areas of EWP. Calculation quantum mechanical correlation of type of λenz/2=l0/n got experimental confirmation, in obedience to which on length of l0 conductor the integer of quantized electronic half-waves is always laid

  16. Production of high energy electrons by irradiation of fs-pulse laser on copper film

    Energy Technology Data Exchange (ETDEWEB)

    Oishi, Yuji; Nayuki, Takuya; Fujii, Takashi; Nemoto, Koshichi [Central Research Inst. of Electric Power Industry, Komae, Tokyo (Japan); Kayoiji, Tsutomu [Tokyo Inst. of Technology, Interdisciplinary Graduate School of Science and Engineering, Yokohama, Kanagawa (Japan); Okano, Yasuaki; Hironaka, Yoichiro; Nakamura, Kazutaka G.; Kondo, Ken-ichi [Tokyo Inst. of Technology, Materials and Structures Laboratory, Yokohama, Kanagawa (Japan)

    2002-07-01

    Fast electrons with energy corresponding to the ponderomotive potential were produced by laser irradiation of 43-fs, 2.7 X 10{sup 18} W/cm{sup 2} on a 30 {mu}m thick copper target. The energy spectra of the electrons were directly measured using a magnetic spectrometer with an imaging plate. The typical temperature was 350 keV for irradiation at 15deg incidence angle. The energy spectra of high-energy photons, which were expected to be produced from the electrons, were also calculated. (author)

  17. Temporal cross-correlation of x-ray free electron and optical lasers using soft x-ray pulse induced transient reflectivity.

    Science.gov (United States)

    Krupin, O; Trigo, M; Schlotter, W F; Beye, M; Sorgenfrei, F; Turner, J J; Reis, D A; Gerken, N; Lee, S; Lee, W S; Hays, G; Acremann, Y; Abbey, B; Coffee, R; Messerschmidt, M; Hau-Riege, S P; Lapertot, G; Lüning, J; Heimann, P; Soufli, R; Fernández-Perea, M; Rowen, M; Holmes, M; Molodtsov, S L; Föhlisch, A; Wurth, W

    2012-05-07

    The recent development of x-ray free electron lasers providing coherent, femtosecond-long pulses of high brilliance and variable energy opens new areas of scientific research in a variety of disciplines such as physics, chemistry, and biology. Pump-probe experimental techniques which observe the temporal evolution of systems after optical or x-ray pulse excitation are one of the main experimental schemes currently in use for ultrafast studies. The key challenge in these experiments is to reliably achieve temporal and spatial overlap of the x-ray and optical pulses. Here we present measurements of the x-ray pulse induced transient change of optical reflectivity from a variety of materials covering the soft x-ray photon energy range from 500eV to 2000eV and outline the use of this technique to establish and characterize temporal synchronization of the optical-laser and FEL x-ray pulses.

  18. Kissing G domains of MnmE monitored by X-ray crystallography and pulse electron paramagnetic resonance spectroscopy.

    Directory of Open Access Journals (Sweden)

    Simon Meyer

    2009-10-01

    Full Text Available MnmE, which is involved in the modification of the wobble position of certain tRNAs, belongs to the expanding class of G proteins activated by nucleotide-dependent dimerization (GADs. Previous models suggested the protein to be a multidomain protein whose G domains contact each other in a nucleotide dependent manner. Here we employ a combined approach of X-ray crystallography and pulse electron paramagnetic resonance (EPR spectroscopy to show that large domain movements are coupled to the G protein cycle of MnmE. The X-ray structures show MnmE to be a constitutive homodimer where the highly mobile G domains face each other in various orientations but are not in close contact as suggested by the GDP-AlF(x structure of the isolated domains. Distance measurements by pulse double electron-electron resonance (DEER spectroscopy show that the G domains adopt an open conformation in the nucleotide free/GDP-bound and an open/closed two-state equilibrium in the GTP-bound state, with maximal distance variations of 18 A. With GDP and AlF(x, which mimic the transition state of the phosphoryl transfer reaction, only the closed conformation is observed. Dimerization of the active sites with GDP-AlF(x requires the presence of specific monovalent cations, thus reflecting the requirements for the GTPase reaction of MnmE. Our results directly demonstrate the nature of the conformational changes MnmE was previously suggested to undergo during its GTPase cycle. They show the nucleotide-dependent dynamic movements of the G domains around two swivel positions relative to the rest of the protein, and they are of crucial importance for understanding the mechanistic principles of this GAD.

  19. Influence of pulse electromagnetic fields on electronic equipment and systems in smart buildings

    Directory of Open Access Journals (Sweden)

    Jacek Paś

    2016-07-01

    Full Text Available The article presents information about the impact of electromagnetic fields’ impulses on technical infrastructure of electronic equipment and systems in intelligent buildings. The use of modern technical solutions in intelligent building management, i.e., human resources control and automation systems, efficient building space management, requires a large number of integrated electronic systems. Impulse interference, lightning or electricity as natural phenomena are among the most responsible for the occurrence of interference in buses, transmission lines systems, electrical installations, equipment and electronic systems used in intelligent buildings. To a large extent, it is associated with catastrophic damages that may occur in electronic devices or in completed systems such as intelligent building, e.g. ICT, security, etc. under the influence of induced voltages and interfering signals’ currents. Keywords: noise, static electricity, lightning

  20. Calibration of an electronic counter and pulse height analyzer for plotting erythrocyte volume spectra.

    Science.gov (United States)

    1963-03-01

    A simple technique is presented for calibrating an electronic system used in the plotting of erythrocyte volume spectra. The calibration factors, once obtained, apparently remain applicable for some time. Precise estimates of calibration factors appe...

  1. Pulse on Pulse

    DEFF Research Database (Denmark)

    Schmidt, Ulrik; Carlson, Merete

    2012-01-01

    of the visitor’s beating heart to the blink of a fragile light bulb, thereby transforming each light bulb into a register of individual life. But at the same time the blinking light bulbs together produce a chaotically flickering light environment composed by various layers of repetitive rhythms, a vibrant...... and pulsating ‘room’. Hence, the visitors in Pulse Room are invited into a complex scenario that continuously oscillates between various aspects of signification (the light bulbs representing individual lives; the pulse itself as the symbolic ‘rhythm of life’) and instants of pure material processuality...... (flickering light bulbs; polyrhythmic layers). Taking our point of departure in a discussion of Gilles Deleuze’s concepts of modulation and signaletic material in relation to electronic media, we examine how the complex orchestration of pulsation between signification and material modulation produces...

  2. Experimental demonstration of electron longitudinal-phase-space linearization by shaping the photoinjector laser pulse.

    Science.gov (United States)

    Penco, G; Danailov, M; Demidovich, A; Allaria, E; De Ninno, G; Di Mitri, S; Fawley, W M; Ferrari, E; Giannessi, L; Trovó, M

    2014-01-31

    Control of the electron-beam longitudinal-phase-space distribution is of crucial importance in a number of accelerator applications, such as linac-driven free-electron lasers, colliders and energy recovery linacs. Some longitudinal-phase-space features produced by nonlinear electron beam self- fields, such as a quadratic energy chirp introduced by geometric longitudinal wakefields in radio-frequency (rf) accelerator structures, cannot be compensated by ordinary tuning of the linac rf phases nor corrected by a single high harmonic accelerating cavity. In this Letter we report an experimental demonstration of the removal of the quadratic energy chirp by properly shaping the electron beam current at the photoinjector. Specifically, a longitudinal ramp in the current distribution at the cathode linearizes the longitudinal wakefields in the downstream linac, resulting in a flat electron current and energy distribution. We present longitudinal-phase-space measurements in this novel configuration compared to those typically obtained without longitudinal current shaping at the FERMI linac.

  3. Controlled Electron Injection into Plasma Accelerators and SpaceCharge Estimates

    Energy Technology Data Exchange (ETDEWEB)

    Fubiani, Gwenael G.J. [Univ. of California, Berkeley, CA (United States)

    2005-09-01

    Plasma based accelerators are capable of producing electron sources which are ultra-compact (a few microns) and high energies (up to hundreds of MeVs) in much shorter distances than conventional accelerators. This is due to the large longitudinal electric field that can be excited without the limitation of breakdown as in RF structures.The characteristic scale length of the accelerating field is the plasma wavelength and for typical densities ranging from 1018 - 1019 cm-3, the accelerating fields and scale length can hence be on the order of 10-100GV/m and 10-40 μm, respectively. The production of quasimonoenergetic beams was recently obtained in a regime relying on self-trapping of background plasma electrons, using a single laser pulse for wakefield generation. In this dissertation, we study the controlled injection via the beating of two lasers (the pump laser pulse creating the plasma wave and a second beam being propagated in opposite direction) which induce a localized injection of background plasma electrons. The aim of this dissertation is to describe in detail the physics of optical injection using two lasers, the characteristics of the electron beams produced (the micrometer scale plasma wavelength can result in femtosecond and even attosecond bunches) as well as a concise estimate of the effects of space charge on the dynamics of an ultra-dense electron bunch with a large energy spread.

  4. Time-resolved electron thermal conduction by probing of plasma formation in transparent solids with high power subpicosecond laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Vu, Brian -Tinh Van [Univ. of California, Davis, CA (United States)

    1994-02-01

    This dissertation work includes a series of experimental measurements in a search for better understanding of high temperature (104-106K) and high density plasmas (1022-1024cm-3) produced by irradiating a transparent solid target with high intensity (1013 - 1015W/cm2) and subpicosecond (10-12-10-13s) laser pulses. Experimentally, pump and probe schemes with both frontside (vacuum-plasma side) and backside (plasma-bulk material side) probes are used to excite and interrogate or probe the plasma evolution, thereby providing useful insights into the plasma formation mechanisms. A series of different experiments has been carried out so as to characterize plasma parameters and the importance of various nonlinear processes. Experimental evidence shows that electron thermal conduction is supersonic in a time scale of the first picosecond after laser irradiation, so fast that it was often left unresolved in the past. The experimental results from frontside probing demonstrate that upon irradiation with a strong (pump) laser pulse, a thin high temperature (~40eV) super-critical density (~1023/cm3) plasma layer is quickly formed at the target surface which in turn becomes strongly reflective and prevents further transmission of the remainder of the laser pulse. In the bulk region behind the surface, it is also found that a large sub-critical (~1018/cm3) plasma is produced by inverse Bremsstrahlung absorption and collisional ionization. The bulk underdense plasma is evidenced by large absorption of the backside probe light. A simple and analytical model, modified from the avalanche model, for plasma evolution in transparent materials is proposed to explain the experimental results. Elimination of the bulk plasma is then experimentally illustrated by using targets overcoated with highly absorptive films.

  5. Enhancement of electron energy to the multi-GeV regime by a dual-stage laser-wakefield accelerator pumped by petawatt laser pulses.

    Science.gov (United States)

    Kim, Hyung Taek; Pae, Ki Hong; Cha, Hyuk Jin; Kim, I Jong; Yu, Tae Jun; Sung, Jae Hee; Lee, Seong Ku; Jeong, Tae Moon; Lee, Jongmin

    2013-10-18

    Laser-wakefield acceleration offers the promise of a compact electron accelerator for generating a multi-GeV electron beam using the huge field gradient induced by an intense laser pulse, compared to conventional rf accelerators. However, the energy and quality of the electron beam from the laser-wakefield accelerator have been limited by the power of the driving laser pulses and interaction properties in the target medium. Recent progress in laser technology has resulted in the realization of a petawatt (PW) femtosecond laser, which offers new capabilities for research on laser-wakefield acceleration. Here, we present a significant increase in laser-driven electron energy to the multi-GeV level by utilizing a 30-fs, 1-PW laser system. In particular, a dual-stage laser-wakefield acceleration scheme (injector and accelerator scheme) was applied to boost electron energies to over 3 GeV with a single PW laser pulse. Three-dimensional particle-in-cell simulations corroborate the multi-GeV electron generation from the dual-stage laser-wakefield accelerator driven by PW laser pulses.

  6. Wavelength dependence of sub-laser-cycle few-electron dynamics in strong-field multiple ionization

    Energy Technology Data Exchange (ETDEWEB)

    Herrwerth, O; Rudenko, A; Kremer, M; Jesus, V L B de; Fischer, B; Gademann, G; Simeonidis, K; Achtelik, A; Ergler, Th; Feuerstein, B; Schroeter, C D; Moshammer, R; Ullrich, J [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, D-69117 Heidelberg (Germany)], E-mail: Artem.Rudenko@mpi-hd.mpg.de

    2008-02-15

    Recoil-ion momentum distributions for double and triple ionization of Ne and Ar, as well as for double ionization of N{sub 2} molecule by intense (0.3-0.5 PW cm{sup -2}), short ({approx}35-40 fs) laser pulses have been recorded in a so far unexplored long laser-wavelength regime at 1300 nm. Compared to earlier results at 800 nm, the direct (e, ne) ionization pathway during recollision is strongly enhanced manifesting itself in a pronounced double-hump structure in the longitudinal ion momentum spectra not only for Ne, but also surprisingly distinct for Ar and, found for the first time, for molecules. Observed wavelength dependence of the sub-laser-cycle correlated few-electron dynamics might be of paramount importance for possible future applications in attosecond science, in particular, for imaging of ultrafast molecular processes via recollision-induced fragmentation.

  7. Single-pulse femtosecond laser Bessel beams drilling of high-aspect-ratio microholes based on electron dynamics control

    Science.gov (United States)

    Zhao, Weiwei; Li, Xiaowei; Xia, Bo; Yan, Xueliang; Han, Weina; Lu, Yongfeng; Jiang, Lan

    2014-11-01

    Microholes drilling has attracted extensive research efforts for its broad applications in photonics, microfluidics, optical fibers and many other fields. A femtosecond (fs) laser is a promising tool for high-precision materials processing with reduced recast/microcracks and minimized heat affected zones. But there remain many challenges in hole drilling using conventional fs laser with Gaussian beams, such as low aspect ratio and taper effects. We report small-diameter and high-aspect-ratio microholes with taper free drilling in PMMA (polymethyl methacrylate) using single-pulse fs laser Bessel beams. Axicon is used to transform Gaussian beams into Bessel beams, which then irradiate in the sample by a telescope consisting of plano-convex lens and microscope objective. Using this technique, we enhance the aspect ratio of microholes by 55 times as compared with Gaussian beams. We attribute this high aspect ratio and high quality microholes formation to the unique spatial intensity distribution and propagation stability of Bessel beams, which can effectively adjust the transient localized electron density distribution leading to a long and uniform localized-interacted zone. By using the optimized pulse energy and focal depth position, the microholes diameter ranges between 1.4-2.1 μm and the aspect ratio can exceed 460. This efficient technique is of great potentials for fabrication of microphotonics devices and microfluidics.

  8. Theory of molecular nonadiabatic electron dynamics in condensed phases

    Science.gov (United States)

    Takatsuka, Kazuo

    2017-11-01

    In light of the rapid progress of ultrafast chemical dynamics driven by the pulse lasers having width as short as several tens of attoseconds, we herein develop a theory of nonadiabatic electron wavepacket dynamics in condensed phases, with which to directly track the dynamics of electronic-state mixing such as electron transfer in liquid solvents. Toward this goal, we combine a theory of path-branching representation for nonadiabatic electron wavepacket dynamics in vacuum {a mixed quantum-classical representation, Yonehara and Takatsuka [J. Chem. Phys. 129, 134109 (2008)]} and a theory of entropy functional to treat chemical dynamics in condensed phases {a mixed dynamical-statistical representation, Takatsuka and Matsumoto [Phys. Chem. Chem. Phys. 18, 1771 (2016)]}. Difficulty and complexity in the present theoretical procedure arise in embedding the Schrödinger equation into classically treated statistical environment. Nevertheless, the resultant equations of motion for electronic-state mixing due to the intrinsic nonadiabatic interactions and solute-solvent interactions, along with the force matrix that drives nuclear branching paths, both turn out to be clear enough to make it possible to comprehend the physical meanings behind. We also discuss briefly the nonvalidness of naive application of the notion of nonadiabatic transition dynamics among free energy surfaces.

  9. Theory of molecular nonadiabatic electron dynamics in condensed phases.

    Science.gov (United States)

    Takatsuka, Kazuo

    2017-11-07

    In light of the rapid progress of ultrafast chemical dynamics driven by the pulse lasers having width as short as several tens of attoseconds, we herein develop a theory of nonadiabatic electron wavepacket dynamics in condensed phases, with which to directly track the dynamics of electronic-state mixing such as electron transfer in liquid solvents. Toward this goal, we combine a theory of path-branching representation for nonadiabatic electron wavepacket dynamics in vacuum {a mixed quantum-classical representation, Yonehara and Takatsuka [J. Chem. Phys. 129, 134109 (2008)]} and a theory of entropy functional to treat chemical dynamics in condensed phases {a mixed dynamical-statistical representation, Takatsuka and Matsumoto [Phys. Chem. Chem. Phys. 18, 1771 (2016)]}. Difficulty and complexity in the present theoretical procedure arise in embedding the Schrödinger equation into classically treated statistical environment. Nevertheless, the resultant equations of motion for electronic-state mixing due to the intrinsic nonadiabatic interactions and solute-solvent interactions, along with the force matrix that drives nuclear branching paths, both turn out to be clear enough to make it possible to comprehend the physical meanings behind. We also discuss briefly the nonvalidness of naive application of the notion of nonadiabatic transition dynamics among free energy surfaces.

  10. Strengthening effect of nano-scaled precipitates in Ta alloying layer induced by high current pulsed electron beam

    Science.gov (United States)

    Tang, Guangze; Luo, Dian; Fan, Guohua; Ma, Xinxin; Wang, Liqin

    2017-05-01

    In this study, the combination of magnetron sputtering and high current pulsed electron beam are used for surface alloying treatment of Ta film on high speed steel. And the Ta alloying layer is about 6 μm. After tempering treatment, TaC phase forms in Ta alloying layer when the treated temperature is over 823 K. Through the TEM and HRTEM observation, a large amount of nano-scaled precipitates (mean diameter 5-8 nm) form within the δ-Fe grain in Ta alloying layer after tempering treatment and these nano-scaled precipitates are confirmed as TaC particles, which contribute to the strengthening effect of the surface alloying layer. The hardness of tempered alloying layer can reach to 18.1 GPa when the treated temperature is 823 K which increase by 50% comparing with the untreated steel sample before surface alloying treatment.

  11. Improved ethanol production of a newly isolated thermotolerant Saccharomyces cerevisiae strain after high-energy-pulse-electron beam.

    Science.gov (United States)

    Zhang, Q; Fu, Y; Wang, Y; Han, J; Lv, J; Wang, S

    2012-02-01

    To isolate thermotolerant Saccharomyces cerevisiae with high-energy-pulse-electron (HEPE) beam, to optimize the mutation strain fermentation conditions for ethanol production and to conduct a preliminary investigation into the thermotolerant mechanisms. After HEPE beam radiation, the thermotolerant S. cerevisiae strain Y43 was obtained at 45°C. Moreover, the fermentation conditions of mutant Y43 were optimized by L3(3) orthogonal experiment. The optimal glucose content and initial pH for fermentation were 20% g l(-1) and 4·5, respectively; peptone content was the most neglected important factor. Under this condition, ethanol production of Y43 was 83·1 g l(-1) after fermentation for 48 h at 43°C, and ethanol yield was 0·42 g g(-1), which was about 81·5% of the theoretical yield. The results also showed that the trehalose content and the expression of the genes MSN2, SSA3 and TPS1 in Y43 were higher than those in the original strain (YE0) under the same stress conditions. A genetically stable mutant strain with high ethanol yield under heat stress was obtained using HEPE. This mutant may be a suitable candidate for the industrial-scale ethanol production. High-energy-pulse-electron radiation is a new efficient technology in breeding micro-organisms. The mutant obtained in this work has the advantages in industrial ethanol production under thermostress. © 2012 The Authors. Journal of Applied Microbiology © 2012 The Society for Applied Microbiology.

  12. Pulse shapes from electron and photon induced events in segmented high-purity germanium detectors

    CERN Document Server

    Abt, I; Kröninger, K; Liu, J; Liu, X; Majorovits, B

    2007-01-01

    Experiments built to search for neutrinoless double beta-decay are limited in their sensitivity not only by the exposure but also by the amount of background encountered. Radioactive isotopes in the surrounding of the detectors which emit gamma-radiation are expected to be a significant source of background in the GERmanium Detector Array, GERDA. Methods to select electron induced events and discriminate against photon induced events inside a germanium detector are presented in this paper. The methods are based on the analysis of the time structure of the detector response. Data were taken with a segmented GERDA prototype detector. It is shown that the analysis of the time response of the detector can be used to distinguish multiply scattered photons from electrons.

  13. Electron Dynamics During High-Power, Short-Pulsed Laser Interactions with Solids and Interfaces

    Science.gov (United States)

    2016-06-28

    phonon thermal conductivity of ferroelectric solids. The electric fields changed the ferroelastic domain states, which varied the phonon scattering rates...Adamo, C., Ye, L., Huey, B., Lee, S., Schlom, D.G., “Strain field and coherent domain wall effects on thermal conductivity and Kapitza conductance...temperature in bilayer and strain-released PZT thin films via modulation of the domain structure using applied electric fields ,” Electronic Materials

  14. Experimental investigations on the influence of the photocathode laser pulse parameters on the electron bunch quality in an RF-photoelectron source

    Energy Technology Data Exchange (ETDEWEB)

    Haenel, Marc

    2010-07-15

    Free Electron Lasers based on the SASE principle like the European XFEL require electron bunches having peak currents of several kiloamperes as well as very low transverse emittance. While high peak currents can be generated using longitudinal bunch compression techniques, the transverse emittance must have values as low as 1mmmrad already at the source. The development of electron sources fulfilling these demanding specifications is the goal of the Photo Injector Test Facility (PITZ) in DESY, Zeuthen site. The key component of a photoinjector is the electron gun cavity where the electrons bunches are generated and immediately accelerated. The extraction of the electrons is based on the photoelectric effect of the cathode which requires a laser system having special capabilities. In the first part of the thesis, measurements are presented which were performed to investigate whether the laser and the laser transport system fulfill these requirements. The second part of the thesis is dedicated to simulations as well as experimental studies on the impact of the temporal and spatial parameters of the laser pulses on the electron bunch quality. This influence is possible because the response time of the Cs{sub 2}Te photocathode is short compared to the laser pulse duration. Based on these investigations, suggestions for improvements are given and tolerances for the laser pulse properties are defined. (orig.)

  15. Symmetry-constrained Analysis of Pulsed Double Electron-Electron Resonance (DEER) Spectroscopy Reveals the Dynamic Nature of the KcsA Activation Gate

    Science.gov (United States)

    Dalmas, Olivier; Hyde, H. Clark; Hulse, Raymond E.; Perozo, Eduardo

    2013-01-01

    Distance determination from an echo intensity modulation obtained by pulsed double electron-electron resonance (DEER) experiment is a mathematically ill-posed problem. Tikhonov regularization yields distance distributions that can be difficult to interpret, especially in system with multiple discrete distance distributions. Here, we show that by using geometric fit constraints in symmetric homo-oligomeric protein systems, we were able to increase the accuracy of a model-based fit solution based on a sum of Gaussian distributions. Our approach was validated on two different ion channels of known oligomeric states, KcsA (a tetramer) and CorA (a pentamer). Statistical analysis of the resulting fits was integrated within our method to help the experimenter evaluate the significance of a symmetry-constrained vs. standard model distribution fit and to examine multi-distance confidence regions. This approach was used to quantitatively evaluate the role of the C-terminal domain (CTD) on the flexibility and conformation of the activation gate of the K+ channel KcsA. Our analysis reveals a significant increase in the dynamics of the inner bundle gate upon opening. Also, it explicitly demonstrates the degree to which the CTD restricts the motion of the lower gate at rest and during activation gating. PMID:22946877

  16. Electronic transport in highly conducting Si-doped ZnO thin films prepared by pulsed laser deposition

    Energy Technology Data Exchange (ETDEWEB)

    Kuznetsov, Vladimir L.; Vai, Alex T.; Edwards, Peter P., E-mail: peter.edwards@chem.ox.ac.uk [Department of Chemistry, Inorganic Chemistry Laboratory, University of Oxford, Oxford OX1 3QR (United Kingdom); Al-Mamouri, Malek; Stuart Abell, J. [Department of Metallurgy and Materials, University of Birmingham, Birmingham B15 2TT (United Kingdom); Pepper, Michael [Department of Electronic and Electrical Engineering, University College London, London WC1E 7JE (United Kingdom)

    2015-12-07

    Highly conducting (ρ = 3.9 × 10{sup −4} Ωcm) and transparent (83%) polycrystalline Si-doped ZnO (SiZO) thin films have been deposited onto borosilicate glass substrates by pulsed laser deposition from (ZnO){sub 1−x}(SiO{sub 2}){sub x} (0 ≤ x ≤ 0.05) ceramic targets prepared using a sol-gel technique. Along with their structural, chemical, and optical properties, the electronic transport within these SiZO samples has been investigated as a function of silicon doping level and temperature. Measurements made between 80 and 350 K reveal an almost temperature-independent carrier concentration consistent with degenerate metallic conduction in all of these samples. The temperature-dependent Hall mobility has been modeled by considering the varying contribution of grain boundary and electron-phonon scattering in samples with different nominal silicon concentrations.

  17. Tailoring the pulse shape to efficiently populate atomic electron metastable states in a relativistically intense high-frequency laser field

    Science.gov (United States)

    Emelin, M. Yu.; Smirnov, L. A.; Ryabikin, M. Yu.

    2017-10-01

    The results of both quantum-mechanical numerical calculations beyond the electric dipole approximation and relativistic classical Monte Carlo simulations are presented for a ground-state hydrogen atom exposed to a high-frequency circularly polarized laser field in a wide intensity range. The persistence of the light-induced metastable bound states well into the relativistic regime of laser-atom interaction is demonstrated. The feasibility of high-efficiency electron trapping into these metastable states is examined in the frame of a simple two-stage scenario for a laser field turning on. The optimal parameters of the laser pulse front are found, which provide an optimal balance between the needs to achieve as quickly as possible the higher intensities, for which the decay rate of the metastable states is lower, and to ensure sufficient adiabaticity of the field turning on to avoid the unwanted "shake-off" processes. As a result, more than 60% probability of electron trapping into the metastable states in a relativistically intense high-frequency laser field is demonstrated.

  18. Transform-limited x-ray pulse generation from a high-brightness self-amplified spontaneous-emission free-electron laser.

    Science.gov (United States)

    McNeil, B W J; Thompson, N R; Dunning, D J

    2013-03-29

    A method to achieve high-brightness self-amplified spontaneous emission (HB-SASE) in the free-electron laser (FEL) is described. The method uses repeated nonequal electron beam delays to delocalize the collective FEL interaction and break the radiation coherence length dependence on the FEL cooperation length. The method requires no external seeding or photon optics and so is applicable at any wavelength or repetition rate. It is demonstrated, using linear theory and numerical simulations, that the radiation coherence length can be increased by approximately 2 orders of magnitude over SASE with a corresponding increase in spectral brightness. Examples are shown of HB-SASE generating transform-limited FEL pulses in the soft x-ray and near transform-limited pulses in the hard x-ray. Such pulses may greatly benefit existing applications and may also open up new areas of scientific research.

  19. Electron self-injection for the acceleration in laser-pulse-wakes in the presence of a `strong' external magnetic field

    OpenAIRE

    Zhidkov, A.; Hosokai, T.; Masuda, S.; Oishi, Y.; Fujii, T.; Kodama, R.

    2012-01-01

    An external static magnetic field with its strength B~10T may result in the laser wake wave-breaking upon changing the electron motion in the vicinity of maximal density ramp of a wave period. This, as shown by numerical simulations, can change the resonance character of the electron self-injection in the laser wake-field; a total charge loaded in the acceleration phase of laser pulse wake can be controlled by a proper choice of the magnetic field strength.

  20. Radiation oxygen biology with pulse electron paramagnetic resonance imaging in animal tumors.

    Science.gov (United States)

    Redler, Gage; Elas, Martyna; Epel, Boris; Barth, Eugene D; Halpern, Howard J

    2013-01-01

    The reduced oxygen in tumors (hypoxia) generates radiation resistance and limits tumor control probability (TCP) at radiation doses without significant normal tissue complication. Modern radiation therapy delivery with intensity-modulated radiation therapy (IMRT) enables complex, high-dose gradient patterns, which avoid sensitive human tissues and organs. EPR oxygen images may allow selection of more resistant parts of a tumor to which to deliver more radiation dose to enhance TCP. EPR O2 images are obtained using injected narrow-line, low relaxation rate trityl spin probes that enable pulse radiofrequency EPR O2 images of tumors in the legs of mice, rats, and rabbits, the latter exceeding 4 cm in size. Low relaxation rates of trityls have enabled novel T1-, rather than T2-, based oximetry, which provides near absolute pO2 imaging. Tomographic image formation and filtered back projection reconstruction are used to generate these images with fixed, linear stepped gradients. Images obtained both with T2 and T1 oximetric images have demonstrated the complex in vivo mechanism explaining the unexpected efficacy of TNFerade, a radiation-inducible adenoviral construct to locally produce TNF-induced vascular as well as radiation damage [1, 2]. The unexpected efficacy of large-dose radiation fractions is seen to be due to an interaction between host microvasculature and tumor cells producing a prompt (15 min) postradiation hypoxia, paralyzing tumor cell repair, and sensitizing tumors. Finally, cure of tumors treated to a single 50 % control dose shows a significant dependence on EPR O2 image hypoxic fractions, best shown with the fraction of voxels less than 10 Torr (HF10). We show that these O2 images provide a quantitative basis for measuring tumor and normal tissue response to abnormally low O2 levels. Measurements of vascular endothelial growth factor (VEGF) production in a specific syngeneic mouse fibrosarcoma, FSa versus fraction of tissue voxels with pO2 less than 10

  1. Electron dynamics and optical properties modulation of monolayer MoS{sub 2} by femtosecond laser pulse: a simulation using time-dependent density functional theory

    Energy Technology Data Exchange (ETDEWEB)

    Su, Xiaoxing; Jiang, Lan [Beijing Institute of Technology, Laser Micro/Nano Fabrication Laboratory, School of Mechanical Engineering, Beijing (China); Wang, Feng [Beijing Institute of Technology, School of Physics, Beijing (China); Su, Gaoshi [Beijing Institute of Technology, School of Mechatronical Engineering, Beijing (China); Qu, Liangti [Beijing Institute of Technology, Key Laboratory of Cluster Science, Ministry of Education, School of Chemistry, Beijing (China); Lu, Yongfeng [University of Nebraska-Lincoln, Department of Electrical Engineering, Lincoln, NE (United States)

    2017-07-15

    In this study, we adopted time-dependent density functional theory to investigate the optical properties of monolayer MoS{sub 2} and the effect of intense few-cycle femtosecond laser pulses on these properties. The electron dynamics of monolayer MoS{sub 2} under few-cycle and multi-cycle laser irradiation were described. The polarization direction of the laser had a marked effect on the energy absorption and electronic excitation of monolayer MoS{sub 2} because of anisotropy. Change in the polarization direction of few-cycle pulse changed the absorbed energy by a factor over 4000. Few-cycle pulse showed a higher sensitivity to the electronic property of material than multi-cycle pulse. The modulation of the dielectric properties of the material was observed on the femtosecond time scale. The negative divergence appeared in the real part of the function at low frequencies and photoinduced blue shift occurred due to Burstein-Moss effect. The irradiation of femtosecond laser caused the dielectric response within the infrared region and introduced anisotropy to the in-plane optical properties. Laser-based engineering of optical properties through controlling transient electron dynamics expands the functionality of MoS{sub 2} and has potential applications in direction-dependent optoelectronic devices. (orig.)

  2. Electron dynamics and optical properties modulation of monolayer MoS2 by femtosecond laser pulse: a simulation using time-dependent density functional theory

    Science.gov (United States)

    Su, Xiaoxing; Jiang, Lan; Wang, Feng; Su, Gaoshi; Qu, Liangti; Lu, Yongfeng

    2017-07-01

    In this study, we adopted time-dependent density functional theory to investigate the optical properties of monolayer MoS2 and the effect of intense few-cycle femtosecond laser pulses on these properties. The electron dynamics of monolayer MoS2 under few-cycle and multi-cycle laser irradiation were described. The polarization direction of the laser had a marked effect on the energy absorption and electronic excitation of monolayer MoS2 because of anisotropy. Change in the polarization direction of few-cycle pulse changed the absorbed energy by a factor over 4000. Few-cycle pulse showed a higher sensitivity to the electronic property of material than multi-cycle pulse. The modulation of the dielectric properties of the material was observed on the femtosecond time scale. The negative divergence appeared in the real part of the function at low frequencies and photoinduced blue shift occurred due to Burstein-Moss effect. The irradiation of femtosecond laser caused the dielectric response within the infrared region and introduced anisotropy to the in-plane optical properties. Laser-based engineering of optical properties through controlling transient electron dynamics expands the functionality of MoS2 and has potential applications in direction-dependent optoelectronic devices.

  3. Distinguishing Between Electrons and γ-Rays in Experiment TGV Using a Pulse Rise Time

    Science.gov (United States)

    Čermák, P.; Štekl, I.; Beneš, P.; Brudanin, V. B.; Rukhadze, N. I.; Egorov, V. G.; Kovalenko, V. E.; Kovalík, A.; Pismenniy, R.; Salamatin, A. V.; Timkin, V.; Vylov, Ts.; Vénos, D.

    2002-04-01

    The TGV (Telescope Germanium Vertical) collaboration is interested in the measurement of double-beta decay of 48Ca (TGV I) and 106Cd (TGV II). The background in the experiment TGV I has been suppressed by several methods. One of them was based on distinguishing between electrons and -rays due to the different rise time of the signals obtained from semiconductor detector. Two experimental setups have been tested, the first one used a charge-sensitive analog-to-digital converter, while the second one utilized digital oscilloscope. The reduction of the background counting rate (due to -rays) in single HPGe detector by a factor of (1.4-3.8) was reached.

  4. Light-Induced Structures in Attosecond Transient Absorption Spectroscopy of Molecules

    CERN Document Server

    Bækhøj, Jens E

    2015-01-01

    The nature of light-induced structures in attosecond transient absorption spectroscopy of molecular systems is investigated theoretically. It is shown how nuclear dynamics affect these structures. We find that a theoretical three-surface model captures the main characteristics in the calculated spectra. Based on this model, nuclear dynamics is divided into different categories, each category having unique signatures in the absorption spectra. Finally, we discuss the possibility for experimental observation of light-induced structures in molecules.

  5. SIMULATION OF FORWARD AND BACKWARD WAVES EVOLUTION OF FEW-CYCLE PULSES PROPAGATING IN AN OPTICAL WAVEGUIDE WITH DISPERSION AND CUBIC NONLINEARITY OF ELECTRONIC AND ELECTRONIC-VIBRATION NATURE

    Directory of Open Access Journals (Sweden)

    L. S. Konev

    2015-09-01

    Full Text Available Numerical method for calculation of forward and backward waves of intense few-cycle laser pulses propagating in an optical waveguide with dispersion and cubic nonlinearity of electronic and electronic-vibration nature is described. Simulations made with the implemented algorithm show that accounting for Raman nonlinearity does not lead to qualitative changes in behavior of the backward wave. Speaking about quantitative changes, the increase of efficiency of energy transfer from the forward wave to the backward wave is observed. Presented method can be also used to simulate interaction of counterpropagating pulses.

  6. Characterization of temporal coherence of hard X-ray free-electron laser pulses with single-shot interferograms

    Directory of Open Access Journals (Sweden)

    Taito Osaka

    2017-11-01

    Full Text Available Temporal coherence is one of the most fundamental characteristics of light, connecting to spectral information through the Fourier transform relationship between time and frequency. Interferometers with a variable path-length difference (PLD between the two branches have widely been employed to characterize temporal coherence properties for broad spectral regimes. Hard X-ray interferometers reported previously, however, have strict limitations in their operational photon energies, due to the specific optical layouts utilized to satisfy the stringent requirement for extreme stability of the PLD at sub-ångström scales. The work presented here characterizes the temporal coherence of hard X-ray free-electron laser (XFEL pulses by capturing single-shot interferograms. Since the stability requirement is drastically relieved with this approach, it was possible to build a versatile hard X-ray interferometer composed of six separate optical elements to cover a wide photon energy range from 6.5 to 11.5 keV while providing a large variable delay time of up to 47 ps at 10 keV. A high visibility of up to 0.55 was observed at a photon energy of 10 keV. The visibility measurement as a function of time delay reveals a mean coherence time of 5.9 ± 0.7 fs, which agrees with that expected from the single-shot spectral information. This is the first result of characterizing the temporal coherence of XFEL pulses in the hard X-ray regime and is an important milestone towards ultra-high energy resolutions at micro-electronvolt levels in time-domain X-ray spectroscopy, which will open up new opportunities for revealing dynamic properties in diverse systems on timescales from femtoseconds to nanoseconds, associated with fluctuations from ångström to nanometre spatial scales.

  7. Amplification of picosecond pulse by electron-beam pumped KrF laser amplifiers. Denshi beam reiki KrF laser zofukuki ni yoru piko byo pulse no zofuku

    Energy Technology Data Exchange (ETDEWEB)

    Okuda, I.; Tomie, T.; Owadano, Y.; Yano, M. (Electrotechnical Laboratory, Tsukuba (Japan))

    1991-08-20

    Experiments on the amplification of a picosecond pulse by electron-beam pumped KrF laser amplifiers were carried out for the purpose of its application to the field such as excitation light source for soft X-ray laser which requires large energy besides peak power. The picosecond pulse was amplified by a discharge pumped KrF amplifier and two electron-beam pumped KrF amplifiers(at the middle stage and the final stage). The energy of 4J, which was the largest energy for short pulse excimer laser so far, was obtained by these devices. About 90% of the window area of the final amplifier with 29cm diameter was filled by the input beam, and energy density of the picosecond beam reached 3.9 times saturation energy density. Measured energy of amplified spontaneous emission(ASE) showed good agreement with the theoretically estimated value. Most of ASE was derived from the discharge pumped laser as the first amplifier. As for the focused power density, the power density ratio of the picosecond pulse to ASE was estimated to be as large as 10{sup 5}. 11 refs., 4 figs.

  8. Low emittance electron beam generation from a laser wakefield accelerator using two laser pulses with different wavelengths

    Directory of Open Access Journals (Sweden)

    X. L. Xu

    2014-06-01

    Full Text Available Ionization injection triggered by short wavelength laser pulses inside a nonlinear wakefield driven by a longer wavelength laser is examined via multidimensional particle-in-cell simulations. We find that very bright electron beams can be generated through this two-color scheme in either collinear propagating or transverse colliding geometry. For a fixed laser intensity I, lasers with longer/shorter wavelength λ have larger/smaller ponderomotive potential (∝Iλ^{2}. The two-color scheme utilizes this property to separate the injection process from the wakefield excitation process. Very strong wakes can be generated at relatively low laser intensities by using a longer wavelength laser driver (e.g., a 10  μm CO_{2} laser due to its very large ponderomotive potential. On the other hand, a short wavelength laser can produce electrons with very small residual momenta (p_{⊥}∼a_{0}∼sqrt[I]λ inside the wake, leading to electron beams with very small normalized emittances (tens of nm. Using particle-in-cell simulations we show that a ∼10  fs electron beam with ∼4  pC of charge and a normalized emittance of ∼50  nm can be generated by combining a 10  μm driving laser with a 400 nm injection laser, which is an improvement of more than 1 order of magnitude compared to the typical results obtained when a single wavelength laser is used for both the wake formation and ionization injection. With the transverse colliding geometry, simulations show that similarly low emittance and much lower slice energy spread (∼30  keV, comparing with the typical value of few MeV in the longitudinal injection scheme can be simultaneously obtained for electron beams with a few pC charge. Such low slice energy spread may have significant advantages in applications relevant to future coherent light sources driven by plasma accelerators.

  9. Integration of digital signal processing technologies with pulsed electron paramagnetic resonance imaging

    Science.gov (United States)

    Pursley, Randall H.; Salem, Ghadi; Devasahayam, Nallathamby; Subramanian, Sankaran; Koscielniak, Janusz; Krishna, Murali C.; Pohida, Thomas J.

    2006-01-01

    The integration of modern data acquisition and digital signal processing (DSP) technologies with Fourier transform electron paramagnetic resonance (FT-EPR) imaging at radiofrequencies (RF) is described. The FT-EPR system operates at a Larmor frequency (Lf) of 300 MHz to facilitate in vivo studies. This relatively low frequency Lf, in conjunction with our ~10 MHz signal bandwidth, enables the use of direct free induction decay time-locked subsampling (TLSS). This particular technique provides advantages by eliminating the traditional analog intermediate frequency downconversion stage along with the corresponding noise sources. TLSS also results in manageable sample rates that facilitate the design of DSP-based data acquisition and image processing platforms. More specifically, we utilize a high-speed field programmable gate array (FPGA) and a DSP processor to perform advanced real-time signal and image processing. The migration to a DSP-based configuration offers the benefits of improved EPR system performance, as well as increased adaptability to various EPR system configurations (i.e., software configurable systems instead of hardware reconfigurations). The required modifications to the FT-EPR system design are described, with focus on the addition of DSP technologies including the application-specific hardware, software, and firmware developed for the FPGA and DSP processor. The first results of using real-time DSP technologies in conjunction with direct detection bandpass sampling to implement EPR imaging at RF frequencies are presented. PMID:16243552

  10. Integration of digital signal processing technologies with pulsed electron paramagnetic resonance imaging.

    Science.gov (United States)

    Pursley, Randall H; Salem, Ghadi; Devasahayam, Nallathamby; Subramanian, Sankaran; Koscielniak, Janusz; Krishna, Murali C; Pohida, Thomas J

    2006-02-01

    The integration of modern data acquisition and digital signal processing (DSP) technologies with Fourier transform electron paramagnetic resonance (FT-EPR) imaging at radiofrequencies (RF) is described. The FT-EPR system operates at a Larmor frequency (L(f)) of 300MHz to facilitate in vivo studies. This relatively low frequency L(f), in conjunction with our approximately 10MHz signal bandwidth, enables the use of direct free induction decay time-locked subsampling (TLSS). This particular technique provides advantages by eliminating the traditional analog intermediate frequency downconversion stage along with the corresponding noise sources. TLSS also results in manageable sample rates that facilitate the design of DSP-based data acquisition and image processing platforms. More specifically, we utilize a high-speed field programmable gate array (FPGA) and a DSP processor to perform advanced real-time signal and image processing. The migration to a DSP-based configuration offers the benefits of improved EPR system performance, as well as increased adaptability to various EPR system configurations (i.e., software configurable systems instead of hardware reconfigurations). The required modifications to the FT-EPR system design are described, with focus on the addition of DSP technologies including the application-specific hardware, software, and firmware developed for the FPGA and DSP processor. The first results of using real-time DSP technologies in conjunction with direct detection bandpass sampling to implement EPR imaging at RF frequencies are presented.

  11. Broadband 2D electronic spectrometer using white light and pulse shaping: noise and signal evaluation at 1 and 100 kHz.

    Science.gov (United States)

    Kearns, Nicholas M; Mehlenbacher, Randy D; Jones, Andrew C; Zanni, Martin T

    2017-04-03

    We have developed a broad bandwidth two-dimensional electronic spectrometer that operates shot-to-shot at repetition rates up to 100 kHz using an acousto-optic pulse shaper. It is called a two-dimensional white-light (2D-WL) spectrometer because the input is white-light supercontinuum. Methods for 100 kHz data collection are studied to understand how laser noise is incorporated into 2D spectra during measurement. At 100 kHz, shot-to-shot scanning of the delays and phases of the pulses in the pulse sequence produces a 2D spectrum 13-times faster and with the same signal-to-noise as using mechanical stages and a chopper. Comparing 100 to 1 kHz repetition rates, data acquisition time is decreased by a factor of 200, which is beyond the improvement expected by the repetition rates alone due to reduction in 1/f noise. These improvements arise because shot-to-shot readout and modulation of the pulse train at 100 kHz enables the electronic coherences to be measured faster than the decay in correlation between laser intensities. Using white light supercontinuum for the pump and probe pulses produces high signal-to-noise spectra on samples with optical densities 200 nm bandwidth.

  12. Femtosecond few- to single-electron point-projection microscopy for nanoscale dynamic imaging

    Directory of Open Access Journals (Sweden)

    A. R. Bainbridge

    2016-03-01

    Full Text Available Femtosecond electron microscopy produces real-space images of matter in a series of ultrafast snapshots. Pulses of electrons self-disperse under space-charge broadening, so without compression, the ideal operation mode is a single electron per pulse. Here, we demonstrate femtosecond single-electron point projection microscopy (fs-ePPM in a laser-pump fs-e-probe configuration. The electrons have an energy of only 150 eV and take tens of picoseconds to propagate to the object under study. Nonetheless, we achieve a temporal resolution with a standard deviation of 114 fs (equivalent to a full-width at half-maximum of 269 ± 40 fs combined with a spatial resolution of 100 nm, applied to a localized region of charge at the apex of a nanoscale metal tip induced by 30 fs 800 nm laser pulses at 50 kHz. These observations demonstrate real-space imaging of reversible processes, such as tracking charge distributions, is feasible whilst maintaining femtosecond resolution. Our findings could find application as a characterization method, which, depending on geometry, could resolve tens of femtoseconds and tens of nanometres. Dynamically imaging electric and magnetic fields and charge distributions on sub-micron length scales opens new avenues of ultrafast dynamics. Furthermore, through the use of active compression, such pulses are an ideal seed for few-femtosecond to attosecond imaging applications which will access sub-optical cycle processes in nanoplasmonics.

  13. Change of texture, microdeformation and hardness in surface layer of TiNi alloy depending on the number of pulses of electron beam effects

    Energy Technology Data Exchange (ETDEWEB)

    Meisner, L. L., E-mail: llm@ispms.tsc.ru; Meisner, S. N., E-mail: msn@ispms.tsc.ru [Institute of Strength Physics and Materials Science SB RAS, Tomsk, 634055 (Russian Federation); National Research Tomsk State University, Tomsk, 634050 (Russian Federation); Markov, A. B., E-mail: a.markov@hq.tsc.ru; Yakovlev, E. V., E-mail: yakovev@lve.hcei.tsc.ru; Ozur, G. E., E-mail: ozur@lve.hcei.tsc.ru [Institute of High Current Electronics SB RAS, Tomsk, 634055 (Russian Federation); Rotshtein, V. P., E-mail: vrotshtein@yahoo.com [Institute of Strength Physics and Materials Science SB RAS, Tomsk, 634055 (Russian Federation); Tomsk State Pedagogical University, Tomsk, 634050 (Russian Federation); Mironov, Yu. P., E-mail: myp@ispms.tsc.ru [Institute of Strength Physics and Materials Science SB RAS, Tomsk, 634055 (Russian Federation)

    2015-10-27

    This work comprises a study of the influence of the pulse number of low-energy high-current electron beam (LEHCEB) exposure on the value and character of distribution of residual elastic stresses, texturing effects and the relationship between structural-phase states and physical and mechanical properties of the modified surface layers of TiNi alloy. LEHCEB processing of the surface of TiNi samples was carried out using a RITM-SP [3] installation. Energy density of electron beam was constant at E{sub s} = 3.9 ± 0.5 J/cm{sup 2}; pulse duration was 2.8 ± 0.3 μs. The number of pulses in the series was changeable, (n = 2–128). It was shown that as the result of multiple LEHCEB processing of TiNi samples, hierarchically organized multilayer structure is formed in the surface layer. The residual stress field of planar type is formed in the modified surface layer as following: in the direction of the normal to the surface the strain component ε{sub ⊥} < 0 (compressing strain), and in a direction parallel to the surface, the strain component ε{sub ||} > 0 (tensile deformation). Texturing effects and the level of residual stresses after LEHCEB processing of TiNi samples with equal energy density of electron beam (∼3.8 J/cm{sup 2}) depend on the number of pulses and increase with the rise of n > 10.

  14. A pulsed electron-photon fluorescence diagnostic technique for temperature and specie concentration measurement at points in relatively dense, unseedded air flows

    Science.gov (United States)

    Muntz, E. P.; Kunc, J. A.; Erwin, D. A.

    1987-01-01

    An analysis is presented on the use of the fluorescence stimulated by combined pulsed electron and photon beams for the study of gas flows up to densities equivalent to an altitude of about 20 km (number density of about 3 x 10 to the 18th/cu cm). The electron beam acts as a pump, requiring no seed gas, to provide a localized concentration of ions or excited state neutrals that can be probed by saturation optical pulses. A short pulse (10ns) electron beam can be used by itself to provide effectively quench-free emission up to number densities of around 10 to the 18th/cm, but is is difficult to maintain satisfactory spatial resolution at this high density. The use of a nearly simultaneous strong optical pulse increases the flexibility of the diagnostic technique, permitting use at densities greater than 10 to the 18th/cu cm with good spatial resolution. The use of flash X-ray sources combined with optical probing also appears promising for densities above 10 to the 19th/cu cm.

  15. Hybrid simulation of electron energy distributions and plasma characteristics in pulsed RF CCP sustained in Ar and SiH4/Ar discharges

    Science.gov (United States)

    Wang, Xi-Feng; Jia, Wen-Zhu; Song, Yuan-Hong; Zhang, Ying-Ying; Dai, Zhong-Ling; Wang, You-Nian

    2017-11-01

    Pulsed-discharge plasmas offer great advantages in deposition of silicon-based films due to the fact that they can suppress cluster agglomeration, moderate the energy of bombarding ions, and prolong the species' diffusion time on the substrate. In this work, a one-dimensional fluid/Monte-Carlo hybrid model is applied to study pulse modulated radio-frequency (RF) plasmas sustained in capacitively coupled Ar and SiH4/Ar discharges. First, the electron energy distributions in pulsed Ar and SiH4/Ar plasmas have been investigated and compared under identical discharge-circuit conditions. The electron energy distribution function (EEDF) in Ar discharge exhibits a familiar bi-Maxwellian shape during the power-on phase of the pulse, while a more complex (resembling a multi-Maxwellian) distribution with extra inflection points at lower energies is observed in the case of the SiH4/Ar mixture. These features become more prominent with the increasing fraction of SiH4 in the gas mixture. The difference in the shape of the EEDF (which is pronounced inside the plasma but not in the RF sheath where electron heating occurs) is mainly attributed to the electron-impact excitations of SiH4. During the power-off phase of the pulse, the EEDFs in both Ar and SiH4/Ar discharges evolve into bi-Maxwellian shapes, with shrinking high energy tails. Furthermore, the parameter of ion species in the case of SiH4/Ar discharge is strongly modulated by pulsing. For positive ions, such as SiH3+ and Si2H4+ , the particle fluxes overshoot at the beginning of the power-on interval. Meanwhile, for negative ions such as SiH2- and SiH3- , density profiles observed between the electrodes are saddle-shaped due to the repulsion by the self-bias electric field as it builds up. During the power-off phase, the wall fluxes of SiH2- and SiH3- gradually increase, leading to a significant decrease in the net surface charge density on the driven electrode. Compared with ions, the density of SiH3 is poorly modulated

  16. Pulsed electron paramagnetic resonance study of domain docking in neuronal nitric oxide synthase: the calmodulin and output state perspective.

    Science.gov (United States)

    Astashkin, Andrei V; Chen, Li; Zhou, Xixi; Li, Huiying; Poulos, Thomas L; Liu, Ke Jian; Guillemette, J Guy; Feng, Changjian

    2014-08-28

    The binding of calmodulin (CaM) to neuronal nitric oxide synthase (nNOS) enables formation of the output state of nNOS for nitric oxide production. Essential to NOS function is the geometry and dynamics of CaM docking to the NOS oxygenase domain, but little is known about these details. In the present work, the domain docking in a CaM-bound oxygenase/FMN (oxyFMN) construct of nNOS was investigated using the relaxation-induced dipolar modulation enhancement (RIDME) technique, which is a pulsed electron paramagnetic resonance technique sensitive to the magnetic dipole interaction between the electron spins. A cysteine was introduced at position 110 of CaM, after which a nitroxide spin label was attached at the position. The RIDME study of the magnetic dipole interaction between the spin label and the ferric heme centers in the oxygenase domain of nNOS revealed that, with increasing [Ca(2+)], the concentration of nNOS·CaM complexes increases and reaches a maximum at [Ca(2+)]/[CaM] ≥ 4. The RIDME kinetics of CaM-bound nNOS represented monotonous decays without well-defined oscillations. The analysis of these kinetics based on the structural models for the open and docked states has shown that only about 15 ± 3% of the CaM-bound nNOS is in the docked state at any given time, while the remaining 85 ± 3% of the protein is in the open conformations characterized by a wide distribution of distances between the bound CaM and the oxygenase domain. The results of this investigation are consistent with a model that the Ca(2+)-CaM interaction causes CaM docking with the oxygenase domain. The low population of the docked state indicates that the CaM-controlled docking between the FMN and heme domains is highly dynamic.

  17. The microstructure and properties of tungsten alloying layer on copper by high-current pulse electron beam

    Science.gov (United States)

    Zhang, Conglin; Lv, Peng; Cai, Jie; Peng, Ching-Tun; Jin, Yunxue; Guan, Qingfeng

    2017-11-01

    In this paper, tungsten (W) was chosen to be an alloying element into the surface layer of commercial pure (cp) copper (Cu) to enhance the surface properties after surface alloying by high current pulsed electron beam (HCPEB). After HCPEB irradiation, part of the blended powder was dissolved into the substrate surface to form an alloyed layer, which has defect structures consisting of dislocation cells/walls. The presence of defect structures induced by HCPEB irradiation provides a large amount of paths for W atoms to form solid solution and ultrafine W particles. The surface hardening is ascribed to intense plastic deformation via stress, sub-grain strengthening, along with the alloying elements via precipitation hardening and/or the solid solution strengthening. The corrosion performance, tested in 3.5% NaCl solution, was significantly enhanced after surface alloying. The improvement in corrosion resistance is essentially attributed to the combination of the structure defects and the addition of alloying elements to form more stable passive film.

  18. Determination of iodopropynyl butylcarbamate in cosmetic formulations utilizing pulsed splitless injection, gas chromatography with electron capture detector.

    Science.gov (United States)

    Palmer, Kevin B; LaFon, William; Burford, Mark D

    2017-09-22

    Current analytical methodology for iodopropynyl butylcarbamate (IPBC) analysis focuses on the use of liquid chromatography and mass spectrometer (LC-MS), but the high instrumentation and operator investment required has resulted in the need for a cost effective alternative methodology. Past publications investigating gas chromatography with electron capture detector (GC-ECD) for IPBC quantitation proved largely unsuccessful, likely due to the preservatives limited thermal stability. The use of pulsed injection techniques commonly used for trace analysis of thermally labile pharmaceutical compounds was successfully adapted for IPBC analysis and utilizes the selectivity of GC-ECD analysis. System optimization and sample preparation improvements resulted in substantial performance and reproducibility gains. Cosmetic formulations preserved with IPBC (50-100ppm) were solvated in toluene/isopropyl alcohol and quantified over the 0.3-1.3μg/ml calibration range. The methodology was robust (relative standard deviation 4%), accurate (98% recovery), and sensitive (limit of detection 0.25ng/ml) for use in routine testing of cosmetic formulation preservation. Copyright © 2017 Elsevier B.V. All rights reserved.

  19. Progress on Low-Temperature Pulsed Electron Deposition of CuInGaSe2 Solar Cells

    Directory of Open Access Journals (Sweden)

    Massimo Mazzer

    2016-03-01

    Full Text Available The quest for single-stage deposition of CuInGaSe2 (CIGS is an open race to replace very effective but capital intensive thin film solar cell manufacturing processes like multiple-stage coevaporation or sputtering combined with high pressure selenisation treatments. In this paper the most recent achievements of Low Temperature Pulsed Electron Deposition (LTPED, a novel single stage deposition process by which CIGS can be deposited at 250 °C, are presented and discussed. We show that selenium loss during the film deposition is not a problem with LTPED as good crystalline films are formed very close to the melting temperature of selenium. The mechanism of formation of good ohmic contacts between CIGS and Mo in the absence of any MoSe2 transition layers is also illustrated, followed by a brief summary of the measured characteristics of test solar cells grown by LTPED. The 17% efficiency target achieved by lab-scale CIGS devices without bandgap modulation, antireflection coating or K-doping is considered to be a crucial milestone along the path to the industrial scale-up of LTPED. The paper ends with a brief review of the open scientific and technological issues related to the scale-up and the possible future applications of the new technology.

  20. Diffraction of X-ray free-electron laser femtosecond pulses on single crystals in the Bragg and Laue geometry.

    Science.gov (United States)

    Bushuev, V A

    2008-09-01

    A solution of the problem of dynamical diffraction for X-ray pulses with arbitrary dimensions in the Bragg and Laue cases in a crystal of any thickness and asymmetry coefficient of reflection is presented. Analysis of pulse form and duration transformation in the process of diffraction and propagation in a vacuum is conducted. It is shown that only the symmetrical Bragg case can be used to avoid smearing of reflected pulses.

  1. Influence of potential pulses amplitude sequence in a voltammetric electronic tongue (VET) applied to assess antioxidant capacity in aliso.

    Science.gov (United States)

    Fuentes, Esteban; Alcañiz, Miguel; Contat, Laura; Baldeón, Edwin O; Barat, José M; Grau, Raúl

    2017-06-01

    Four signals configurations were studied, two of them built by small increases of potential and two with bigger increments. The highest current values were obtained when pulses with bigger change of potential were used although the best results were shown by the pulse sequence which included an intermediate pulse before the relevant pulse. A mathematical model based on trolox pattern was developed to predict antioxidant capacity of aliso, employing information obtained from all the electrodes, although model validation could be done only employing the information from gold electrode. Copyright © 2016 Elsevier Ltd. All rights reserved.

  2. Multi-colour pulses from seeded free-electron-lasers: towards the development of non-linear core-level coherent spectroscopies.

    Science.gov (United States)

    Bencivenga, Filippo; Capotondi, Flavio; Casolari, Francesco; Dallari, Francesco; Danailov, Miltcho B; De Ninno, Giovanni; Fausti, Daniele; Kiskinova, Maya; Manfredda, Michele; Masciovecchio, Claudio; Pedersoli, Emanuele

    2014-01-01

    We report on new opportunities for ultrafast science thanks to the use of two-colour extreme ultraviolet (XUV) pulses at the FERMI free electron laser (FEL) facility. The two pulses have been employed to carry out a pioneering FEL-pump/FEL-probe diffraction experiment using a Ti target and tuning the FEL pulses to the M(2/3)-edge in order to explore the dependence of the dielectric constant on the excitation fluence. The future impact that the use of such a two-colour FEL emission will have on the development of ultrafast wave-mixing methods in the XUV/soft X-ray range is addressed and discussed.

  3. Generation of a few femtosecond keV x-ray pulse via interaction of a tightly focused laser copropagating with a relativistic electron bunch

    Directory of Open Access Journals (Sweden)

    Sang-Young Chung

    2011-06-01

    Full Text Available It is demonstrated in a numerical simulation that an intense fs keV x-ray pulse can be generated by the interaction of a tightly focused femtosecond laser copropagating with an electron bunch. In general, the interaction of a loosely focused (focal spot ∼100  μm in diameter laser with a copropagating electron is rather weak so that the radiation is not only weak but also produced in the vicinity of laser wavelength. However, in the case of tight focus (focal spot on the order of wavelength, the radiation characteristics turn out to be drastically different so that a keV x-ray pulse can be produced at high flux. This is due to the nonparaxial fields induced in a tight-focus regime. The radiation characteristics are discussed for different beam waists and electron beam energies. This simulation suggests that the interaction of a tightly focused laser with a copropagating electron bunch can be a unique source for an x-ray pulse of the photon energy from 10 to 100 keV that lasts a few femtoseconds.

  4. Muscle contraction during electro-muscular incapacitation: A comparison between square-wave pulses and the TASER(®) X26 Electronic control device.

    Science.gov (United States)

    Comeaux, James A; Jauchem, James R; Cox, D Duane; Crane, Carrie C; D'Andrea, John A

    2011-01-01

    Electronic control devices (including the Advanced TASER(®) X26 model produced by TASER International) incapacitate individuals by causing muscle contractions. To provide information relevant to development of future potential devices, effects of monophasic square waves with different parameters were compared with those of the X26 electronic control device, using two animal models (frogs and swine). Pulse power, electrical pulse charge, pulse duration, and pulse repetition frequency affected muscle contraction. There was no difference in the charge required, between the square waveform and the X26 waveform, to cause approximately the same muscle-contraction response (in terms of the strength-duration curve). Thus, on the basis of these initial studies, the detailed shape of a waveform may not be important in terms of generating electro-muscular incapacitation. More detailed studies, however, may be required to thoroughly test all potential waveforms to be considered for future use in ECDs. 2010 American Academy of Forensic Sciences. Published 2010. This article is a U.S. Government work and is in the public domain in the U.S.A.

  5. Interaction of electron beams with optical nanostructures and metamaterials: from coherent photon sources towards shaping the wave function

    Science.gov (United States)

    Talebi, Nahid

    2017-10-01

    example to form attosecond electron pulses or chiral electron wave functions.

  6. Surface microstructure and B2 phase structural state induced in NiTi alloy by a high-current pulsed electron beam

    Energy Technology Data Exchange (ETDEWEB)

    Meisner, L.L. [Institute of Strength Physics and Materials Science SB RAS, 2/4 Akademichesky Ave., Tomsk 634021 (Russian Federation); National Research Tomsk State University, 36 Lenin Ave., Tomsk 634036 (Russian Federation); Ostapenko, M.G., E-mail: artifakt@ispms.tsc.ru [Institute of Strength Physics and Materials Science SB RAS, 2/4 Akademichesky Ave., Tomsk 634021 (Russian Federation); National Research Tomsk Polytechnic University, 30 Lenin Ave., Tomsk 634036 (Russian Federation); Lotkov, A.I.; Neiman, A.A. [Institute of Strength Physics and Materials Science SB RAS, 2/4 Akademichesky Ave., Tomsk 634021 (Russian Federation)

    2015-01-01

    Graphical abstract: - Highlights: • Structural states of B2 and B19′ phases in the modified NiTi surface zone were analyzed depending on beam energy density. • The surface structure was examined by XRD analysis and transmission electron microscopy. • The formation of the martensite phase in the surface or intermediate NiTi layers depends on the beam energy density. • The factors responsible for changes in the chemical composition of NiTi surface layers after electron beam treatment were analyzed. - Abstract: In the work, we studied structural phase states in surface layers of electron beam-irradiated nickel-titanium (NiTi) alloy depending on beam energy density. The surface of NiTi specimens was exposed to pulsed irradiation (pulse duration τ = 150 μs, number of pulses N = 5) by a low-energy high-current (I = 70 A) electron beam with surface melting at electron beam energy densities E{sub 1} = 15 J/cm{sup 2}, E{sub 2} = 20 J/cm{sup 2}, and E{sub 3} = 30 J/cm{sup 2}. The surface layer structure was examined by X-ray diffraction analysis and transmission electron microscopy. It is found that in the NiTi specimens irradiated at E ≤ 20 J/cm{sup 2}, the layer that contains a martensite phase resides not on the surface but at some depth from it. In the NiTi specimens irradiated at E{sub 3} = 30 J/cm{sup 2}, the entire modified surface zone is characterized by a two-phase state in which the B19′ phase dominates over the B2 phase. It is supposed that a barrier to B2 → B19′ martensite transformation in the melted NiTi layer irradiated at E ≤ 20 J/cm{sup 2} is high inhomogeneous residual stresses varying with depth from the irradiated surface.

  7. Potential beneficial effects of electron-hole plasmas created in silicon sensors by XFEL-like high intensity pulses for detector development

    Energy Technology Data Exchange (ETDEWEB)

    Weiss, Joel T.; Becker, Julian; Shanks, Katherine S.; Philipp, Hugh T.; Tate, Mark W. [Laboratory of Atomic and Solid State Physics, Cornell University, Ithaca, NY 14853 (United States); Gruner, Sol M., E-mail: smg26@cornell.edu [Laboratory of Atomic and Solid State Physics, Cornell University, Ithaca, NY 14853 (United States); Cornell High Energy Synchrotron Source (CHESS), Cornell University, Ithaca, NY 14853 (United States)

    2016-07-27

    There is a compelling need for a high frame rate imaging detector with a wide dynamic range, from single x-rays/pixel/pulse to >10{sup 6} x-rays/pixel/pulse, that is capable of operating at both x-ray free electron laser (XFEL) and 3rd generation sources with sustained fluxes of > 10{sup 11} x-rays/pixel/s [1, 2, 3]. We propose to meet these requirements with the High Dynamic Range Pixel Array Detector (HDR-PAD) by (a) increasing the speed of charge removal strategies [4], (b) increasing integrator range by implementing adaptive gain [5], and (c) exploiting the extended charge collection times of electron-hole pair plasma clouds that form when a sufficiently large number of x-rays are absorbed in a detector sensor in a short period of time [6]. We have developed a measurement platform similar to the one used in [6] to study the effects of high electron-hole densities in silicon sensors using optical lasers to emulate the conditions found at XFELs. Characterizations of the employed tunable wavelength laser with picosecond pulse duration have shown Gaussian focal spots sizes of 6 ± 1 µm rms over the relevant spectrum and 2 to 3 orders of magnitude increase in available intensity compared to previous measurements presented in [6]. Results from measurements on a typical pixelated silicon diode intended for use with the HDR-PAD (150 µm pixel size, 500 µm thick sensor) are presented.

  8. Hot-electron influence on L-shell spectra of multicharged Kr ions generated in clusters irradiated by femtosecond laser pulses.

    Science.gov (United States)

    Hansen, S B; Shlyaptseva, A S; Faenov, A Y; Skobelev, I Y; Magunov, A I; Pikuz, T A; Blasco, F; Dorchies, F; Stenz, C; Salin, F; Auguste, T; Dobosz, S; Monot, P; D' Oliveira, P; Hulin, S; Safronova, U I; Fournier, K B

    2002-10-01

    Strong L-shell x-ray emission has been obtained from Kr clusters formed in gas jets and irradiated by 60-500-fs laser pulses. Spectral lines from the F-, Ne- Na-, and Mg-like charge states of Kr have been identified from highly resolved x-ray spectra. Spectral line intensities are used in conjunction with a detailed time-dependent collisional-radiative model to diagnose the electron distribution functions of plasmas formed in various gas jet nozzles with various laser pulse durations. It is shown that L-shell spectra formed by relatively long nanosecond-laser pulses can be well described by a steady-state model without hot electrons when opacity effects are included. In contrast, adequate modeling of L-shell spectra from highly transient and inhomogeneous femtosecond-laser plasmas requires including the influence of hot electrons. It is shown that femtosecond-laser interaction with gas jets from conical nozzles produces plasmas with higher ionization balances than plasmas formed by gas jets from Laval nozzles, in agreement with previous work for femtosecond laser interaction with Ar clusters.

  9. Theoretical analysis and simulation of the influence of self-bunching effects and longitudinal space charge effects on the propagation of keV electron bunch produced by a novel S-band Micro-Pulse electron Gun

    Directory of Open Access Journals (Sweden)

    Jifei Zhao

    2016-06-01

    Full Text Available As an important electron source, Micro-Pulse electron Gun (MPG which is qualified for producing high average current, short pulse, low emittance electron bunches steadily holds promise to use as an electron source of Coherent Smith-Purcell Radiation (CSPR, Free Electron Laser (FEL. The stable output of S-band MPG has been achieved in many labs. To establish reliable foundation for the future application of it, the propagation of picosecond electron bunch produced by MPG should be studied in detail. In this article, the MPG which was working on the rising stage of total effective Secondary Electron Yield (SEY curve was introduced. The self-bunching mechanism was discussed in depth both in the multipacting amplifying state and the steady working state. The bunch length broadening induced by the longitudinal space-charge (SC effects was investigated by different theoretical models in different regions. The 2D PIC codes MAGIC and beam dynamic codes TraceWin simulations were also performed in the propagation. The result shows an excellent agreement between the simulation and the theoretical analysis for bunch length evolution.

  10. Pulsed laser-assisted focused electron-beam-induced etching of titanium with XeF2: enhanced reaction rate and precursor transport.

    Science.gov (United States)

    Noh, J H; Fowlkes, J D; Timilsina, R; Stanford, M G; Lewis, B B; Rack, P D

    2015-02-25

    In order to enhance the etch rate of electron-beam-induced etching, we introduce a laser-assisted focused electron-beam-induced etching (LA-FEBIE) process which is a versatile, direct write nanofabrication method that allows nanoscale patterning and editing. The results demonstrate that the titanium electron stimulated etch rate via the XeF2 precursor can be enhanced up to a factor of 6 times with an intermittent pulsed laser assist. The evolution of the etching process is correlated to in situ stage current measurements and scanning electron micrographs as a function of time. The increased etch rate is attributed to photothermally enhanced Ti-F reaction and TiF4 desorption and in some regimes enhanced XeF2 surface diffusion to the reaction zone.

  11. Zero vector potential mechanism of attosecond absorption in strongly relativistic plasmas

    CERN Document Server

    Baeva, T; Robinson, A P L; Norreys, P A

    2010-01-01

    The understanding of the physics of lasermatter interactions in the strongly relativistic regime is of fundamental importance. In this article, a new mechanism of fast electron generation at the vacuum-solid boundary of intense laser pulse interaction with overdense plasma is described. It is one that has no analogue in classical, non-relativistic laser-plasma interactions. Here, conclusive proof is provided that the key contribution to the fast electron generation is given by the zero points of the vector potential. We demonstrate that the new mechanism leads to scalings for the fast electron energy, which explicitly depend on the plasma density, thus providing a new insight into relativistic laser-matter interaction. Furthermore, it is shown that this new mechanism provides the dominant contribution to the interaction by the injection of energy into the overdense plasma delivered by attosecondduration electron bunches. This new understanding will allow the future generation of a single ultra-bright attoseco...

  12. Reconstructing the energy band electronic structure of pulsed laser deposited CZTS thin films intended for solar cell absorber applications

    Energy Technology Data Exchange (ETDEWEB)

    Pandiyan, Rajesh [Institut National de la Recherche Scientifique, Centre-Énergie, Matériaux et Télécommunications, 1650 Blvd. Lionel–Boulet, C.P. 1020, Varennes, QC J3X-1S2 (Canada); Oulad Elhmaidi, Zakaria [Institut National de la Recherche Scientifique, Centre-Énergie, Matériaux et Télécommunications, 1650 Blvd. Lionel–Boulet, C.P. 1020, Varennes, QC J3X-1S2 (Canada); University of Mohammed V, Faculty of Sciences, Materials Physics Laboratory, B.P. 1014 Rabat (Morocco); Sekkat, Zouheir [Optics & Photonics Center, Moroccan Foundation for Advanced Science, Innovation and Research, Rabat (Morocco); Abd-lefdil, Mohammed [University of Mohammed V, Faculty of Sciences, Materials Physics Laboratory, B.P. 1014 Rabat (Morocco); El Khakani, My Ali, E-mail: elkhakani@emt.inrs.ca [Institut National de la Recherche Scientifique, Centre-Énergie, Matériaux et Télécommunications, 1650 Blvd. Lionel–Boulet, C.P. 1020, Varennes, QC J3X-1S2 (Canada)

    2017-02-28

    Highlights: • High quality CZTS thin films grown by means of PLD technique without resorting to any post sulfurization process. • Effect of thermal annealing treatments (in the 200–500 °C range) on the structural, morphological and optoelectronic properties of PLD-CZTS films. • Experimental determination of key optoelectronic parameters (i.e.; E{sub g}, VBM, ϕ, I{sub p}, and χ) enabling the reconstruction of energy band electronic structure of the PLD-CZTS films. • Investigation on the energy band alignments of the heterojunction interface formed between CZTS and both CdS and ZnS buffer layer materials. - Abstract: We report here on the use of pulsed KrF-laser deposition (PLD) technique for the growth of high-quality Cu{sub 2}ZnSnS{sub 4} (CZTS) thin films onto Si, and glass substrates without resorting to any post sulfurization process. The PLD-CZTS films were deposited at room temperature (RT) and then subjected to post annealing at different temperatures ranging from 200 to 500 °C in Argon atmosphere. The X-ray diffraction and Raman spectroscopy confirmed that the PLD films crystallize in the characteristic kesterite CZTS structure regardless of their annealing temperature (T{sub a}), but their crystallinity is much improved for T{sub a} ≥ 400 °C. The PLD-CZTS films were found to exhibit a relatively dense morphology with a surface roughness (RMS) that increases with T{sub a} (from ∼14 nm at RT to 70 nm at T{sub a} = 500 °C with a value around 40 nm for T{sub a} = 300–400 °C). The optical bandgap of the PLD-CZTS films, was derived from UV–vis transmission spectra analysis, and found to decrease from 1.73 eV for non-annealed films to ∼1.58 eV for those annealed at T{sub a} = 300 °C. These band gap values are very close to the optimum value needed for an ideal solar cell absorber. In order to achieve a complete reconstruction of the one-dimensional energy band structure of these PLD-CZTS absorbers, we have combined both XPS and UPS

  13. Protons and electrons generated from a 5-{mu}m thick copper tape target irradiated by s-, circularly-, and p-polarized 55-fs laser pulses

    Energy Technology Data Exchange (ETDEWEB)

    Li, Z. [Advanced Photon Research Center, Japan Atomic Energy Agency, Umeimidai 8-1, Kizu, Kyoto 619-0215 (Japan); National Institute of Radiological Sciences, Anagawa 4-9-1, Inage, Chiba 263-8555 (Japan)], E-mail: lizhong@sinap.ac.cn; Daido, H. [Advanced Photon Research Center, Japan Atomic Energy Agency, Umeimidai 8-1, Kizu, Kyoto 619-0215 (Japan); Fukumi, A. [Advanced Photon Research Center, Japan Atomic Energy Agency, Umeimidai 8-1, Kizu, Kyoto 619-0215 (Japan); National Institute of Radiological Sciences, Anagawa 4-9-1, Inage, Chiba 263-8555 (Japan); Bulanov, S.V.; Sagisaka, A.; Ogura, K.; Yogo, A.; Nishiuchi, M.; Orimo, S.; Mori, M. [Advanced Photon Research Center, Japan Atomic Energy Agency, Umeimidai 8-1, Kizu, Kyoto 619-0215 (Japan); Oishi, Y.; Nayuki, T.; Fujii, T.; Nemoto, K. [Central Research Institute of Electric Power Industry, Nagasaka 2-6-1, Yokosuka, Kanagawa 240-0196 (Japan); Nakamura, S.; Noda, A. [Institute of Chemical Research, Kyoto University, Gokasho, Uji, Kyoto 611-0011 (Japan); Choi, I.W.; Sung, J.H.; Ko, D.-K.; Lee, J. [Advanced Photonics Research Institute, Gwangju Institute of Science and Technology, Gwangju 500-712 (Korea, Republic of)

    2007-10-01

    The angular distribution and energy spectra of energetic protons emitted from a 5-{mu}m thick copper tape target irradiated by p-, circularly-, and s-polarized 55-fs laser pulses with intensity of 8-9x10{sup 18} W/cm{sup 2} are measured. The protons are found in the rear target normal direction while the hot electrons are found in the laser propagation direction. The maximum energy of protons is equal to 1.34 MeV for p-polarized irradiation. The energy spectrum of protons depends strongly on the total amount of electrons but it does not so strongly depend on the electron angular distribution under our experiment conditions. Two-dimensional particle in cell simulations also show the maximal proton acceleration for the p-polarized pulse, less efficient acceleration for the circular polarization, and lower acceleration efficiency in the case of the s-polarization, which is related to the electron acceleration efficiency at the front side of the target.

  14. Statistical approach to tunneling time in attosecond experiments

    Science.gov (United States)

    Demir, Durmuş; Güner, Tuğrul

    2017-11-01

    Tunneling, transport of particles through classically forbidden regions, is a pure quantum phenomenon. It governs numerous phenomena ranging from single-molecule electronics to donor-acceptor transition reactions. The main problem is the absence of a universal method to compute tunneling time. This problem has been attacked in various ways in the literature. Here, in the present work, we show that a statistical approach to the problem, motivated by the imaginary nature of time in the forbidden regions, lead to a novel tunneling time formula which is real and subluminal (in contrast to various known time definitions implying superluminal tunneling). In addition to this, we show explicitly that the entropic time formula is in good agreement with the tunneling time measurements in laser-driven He ionization. Moreover, it sets an accurate range for long-range electron transfer reactions. The entropic time formula is general enough to extend to the photon and phonon tunneling phenomena.

  15. Multi-petahertz electronic metrology.

    Science.gov (United States)

    Garg, M; Zhan, M; Luu, T T; Lakhotia, H; Klostermann, T; Guggenmos, A; Goulielmakis, E

    2016-10-20

    The frequency of electric currents associated with charge carriers moving in the electronic bands of solids determines the speed limit of electronics and thereby that of information and signal processing. The use of light fields to drive electrons promises access to vastly higher frequencies than conventionally used, as electric currents can be induced and manipulated on timescales faster than that of the quantum dephasing of charge carriers in solids. This forms the basis of terahertz (1012 hertz) electronics in artificial superlattices, and has enabled light-based switches and sampling of currents extending in frequency up to a few hundred terahertz. Here we demonstrate the extension of electronic metrology to the multi-petahertz (1015 hertz) frequency range. We use single-cycle intense optical fields (about one volt per ångström) to drive electron motion in the bulk of silicon dioxide, and then probe its dynamics by using attosecond (10-18 seconds) streaking to map the time structure of emerging isolated attosecond extreme ultraviolet transients and their optical driver. The data establish a firm link between the emission of the extreme ultraviolet radiation and the light-induced intraband, phase-coherent electric currents that extend in frequency up to about eight petahertz, and enable access to the dynamic nonlinear conductivity of silicon dioxide. Direct probing, confinement and control of the waveform of intraband currents inside solids on attosecond timescales establish a method of realizing multi-petahertz coherent electronics. We expect this technique to enable new ways of exploring the interplay between electron dynamics and the structure of condensed matter on the atomic scale.

  16. Focusing X-ray free-electron laser pulses using Kirkpatrick-Baez mirrors at the NCI hutch of the PAL-XFEL.

    Science.gov (United States)

    Kim, Jangwoo; Kim, Hyo Yun; Park, Jaehyun; Kim, Sangsoo; Kim, Sunam; Rah, Seungyu; Lim, Jun; Nam, Ki Hyun

    2018-01-01

    The Pohang Accelerator Laboratory X-ray Free-Electron Laser (PAL-XFEL) is a recently commissioned X-ray free-electron laser (XFEL) facility that provides intense ultrashort X-ray pulses based on the self-amplified spontaneous emission process. The nano-crystallography and coherent imaging (NCI) hutch with forward-scattering geometry is located at the hard X-ray beamline of the PAL-XFEL and provides opportunities to perform serial femtosecond crystallography and coherent X-ray diffraction imaging. To produce intense high-density XFEL pulses at the interaction positions between the X-rays and various samples, a microfocusing Kirkpatrick-Baez (KB) mirror system that includes an ultra-precision manipulator has been developed. In this paper, the design of a KB mirror system that focuses the hard XFEL beam onto a fixed sample point of the NCI hutch, which is positioned along the hard XFEL beamline, is described. The focusing system produces a two-dimensional focusing beam at approximately 2 µm scale across the 2-11 keV photon energy range. XFEL pulses of 9.7 keV energy were successfully focused onto an area of size 1.94 µm × 2.08 µm FWHM.

  17. Producing nano-grained and Al-enriched surface microstructure on AZ91 magnesium alloy by high current pulsed electron beam treatment

    Energy Technology Data Exchange (ETDEWEB)

    Hao, Shengzhi, E-mail: ebeam@dlut.edu.cn; Li, Mincai

    2016-05-15

    Highlights: • HCPEB surface treatment was conducted on AZ91 magnesium alloy. • Surface modified microstructure and phase composition were characterized. • Preferential evaporation of Mg and dissolution of Mg{sub 17}Al{sub 12} phase occurred. • Nano-grained and Al-enriched surface layer was produced of depth ∼8 μm. • Surface microhardness and corrosion resistance were improved simultaneously. - Abstract: Surface treatment of AZ91 magnesium alloy was carried out by high current pulsed electron beam (HCPEB) with accelerating voltage 27 kV and energy density 3 J/cm{sup 2}. The surface microstructure and phase composition were characterized by using optical microscope (OM), X-ray diffraction (XRD), and scanning electron microscope (SEM) equipped with energy dispersive spectrometer (EDS). The surface microhardness and corrosion resistance were measured. Under HCPEB treatments, the preferential evaporation of Mg element occurred intensively on irradiated surface and the initial large Mg{sub 17}Al{sub 12} phases were dissolved. The nano-grained and Al-enriched surface modified layer was ultimately formed of depth ∼8 μm. According to the testing results, the surface microhardness increased from 63 to 141 HK after 30 pulses of HCPEB treatment, while the best improvement of corrosion resistance was obtained by 15 pulses of HCPEB treatment with a cathodic current density decreased by two orders of magnitude as compared with the initial AZ91 sample.

  18. Atomic Cluster Ionization and Attosecond Generation at Long Wavelengths

    Science.gov (United States)

    2015-10-31

    very sensitive to the small ellipticity of the driving field due to the modification of the electron trajectory . Figure 3 shows the HHG yield with...of short trajectories for our geometry. Second, the group delay from the cluster and monomer show a striking similarity suggesting that the...this test. In order to further investigate this result, we performed an ellipticity study of the HHG yield. The idea is that if the returning

  19. Standard practice for evaluating performance characteristics of ultrasonic Pulse-Echo testing instruments and systems without the use of electronic measurement instruments

    CERN Document Server

    American Society for Testing and Materials. Philadelphia

    2011-01-01

    1.1 This practice describes procedures for evaluating the following performance characteristics of ultrasonic pulse-echo examination instruments and systems: Horizontal Limit and Linearity; Vertical Limit and Linearity; Resolution - Entry Surface and Far Surface; Sensitivity and Noise; Accuracy of Calibrated Gain Controls. Evaluation of these characteristics is intended to be used for comparing instruments and systems or, by periodic repetition, for detecting long-term changes in the characteristics of a given instrument or system that may be indicative of impending failure, and which, if beyond certain limits, will require corrective maintenance. Instrument characteristics measured in accordance with this practice are expressed in terms that relate to their potential usefulness for ultrasonic testing. Instrument characteristics expressed in purely electronic terms may be measured as described in E1324. 1.2 Ultrasonic examination systems using pulsed-wave trains and A-scan presentation (rf or video) may be ev...

  20. Structural transformations in silicon under exposure by femtosecond laser pulse: role of electron-hole plasma and phonon-phonon anharmonism

    CERN Document Server

    Kudryashov, S I

    2002-01-01

    It is experimentally shown for the first time that by the effect of the feed-up laser pulse of 100 fs duration on the silicon target the consecutive structural transitions of the substance into the new crystalline and liquid metallic phase occur both during the laser pulse feed-up and after 0.1-10 sup 3 ps, depending on the material excitation conditions. The thresholds of the observed structural transitions are determined and the phonon nodes, responsible for therefore, are identified. The structural transitions dynamics in the silicon by the 01.-10 sup 3 ps times is described within the frames of the model of the phonon modes instability, originating due to the plasma electron-hole effect and also due to the intra- and intermode phonon-phonon anharmonic interactions

  1. Response Time-Shortened Zinc Oxide Scintillator for Accurate Single-Shot Synchronization of Extreme Ultraviolet Free-Electron Laser and Short-Pulse Laser

    Science.gov (United States)

    Shimizu, Toshihiko; Yamanoi, Kohei; Sakai, Kohei; Cadatal-Raduban, Marilou; Nakazato, Tomoharu; Sarukura, Nobuhiko; Kano, Masataka; Wakamiya, Akira; Ehrentraut, Dirk; Fukuda, Tsuguo; Nagasono, Mitsuru; Togashi, Tadashi; Matsubara, Shinichi; Tono, Kensuke; Higashiya, Atsushi; Yabashi, Makina; Kimura, Hiroaki; Ohashi, Haruhiko; Ishikawa, Tetsuya

    2011-06-01

    We report an over one-order-of magnitude improvement in the response time of conventional hydrothermal method-grown zinc oxide (ZnO) scintillator by introducing additional quenching channels via intentional indium ion doping. A 3-ps fluorescence decay time constant is achieved, therefore making it the fastest scintillator operating below 100 nm to date. Using this indium-doped ZnO, relative jitter between extreme ultraviolet free electron laser (EUV-FEL) probe and optical pump pulses is evaluated to be less than 3 ps. Moreover, pulses from these sources can be synchronized with 3-ps accuracy through in-situ observation of relative time difference in single-shot base.

  2. The effect of neodymium on the microcracks generated on the Al–17.5Si alloy surface treated by high current pulsed electron beam

    Energy Technology Data Exchange (ETDEWEB)

    Hu, Liang; Gao, Bo, E-mail: gaob@smm.neu.edu.cn; Zhu, Guanglin; Hao, Yi; Sun, Shuchen; Tu, Ganfeng

    2016-02-28

    Graphical abstract: SEM results demonstrate that microcracks are remarkably removed from the Al–17.5Si alloy surface after HCPEB treatment due to Nd element, and they decrease in length at high pulse number, showing a decrease in the stress concentration in the primary Si phase during the cooling process of HCPEB, as shown in Fig. 1. Therefore, the microcrack elimination is attributed to reducing the stress concentration. - Highlights: • The main highlights in this paper are summarized as follows: (1) After adding rare earth Nd, the microcracks are remarkably removed from an Al–17.5Si alloy surface by HCPEB, resulting in an improved corrosion resistance of the alloy surface. (2) A site-fixed observation of SEM is first proposed in HCPEB-treated technology, and a microcrack evolution with increasing pulsed numbers is observed for alloy surfaces using this method. (3) The elimination mechanism of microcracks with rare earth Nd is first presented in the present work. (4) Compound modification of rare earth Nd and HCPEB technology on the Al–17.5Si alloy is first investigated. - Abstract: In the present work, the effect of Nd on the microcracks generated on an Al–17.5Si alloy surface by a high current pulsed electron beam (HCPEB) was investigated. By a newly proposed site-fixed observation, the propagation of microcracks with increasing pulsed numbers first increases and then decreases due to the Nd element. The crack density decreases from 0.0669 mm/mm{sup 2} of 5 pulses to 0.00687 mm/mm{sup 2} of 50 pulses. EPMA analysis results indicate that Nd is uniformly distributed on the HCPEB-treated alloy surface. Nano-silicon particles and nano-Al cellular structures were formed by TEM observation, showing grain refinement of the alloy surface. The microcrack elimination is attributed to a decrease in the stress concentration in the primary Si phase during the cooling process of HCPEB. The electrochemical measurement shows that the corrosion current density

  3. Luminescence characteristics of Xe2Cl excimer molecules under pumping the dense Xe—CCl4 gas mixtures with a pulsed electron beam

    Science.gov (United States)

    Mis'kevich, A. I.; Jinbo, Guo

    2013-05-01

    Temporal and spectral characteristics of the luminescence of dense Xe—CCl4 gas mixtures of different composition, excited by a 5-ns pulsed electron beam, were measured. The energy of the electrons amounted to 150 keV and the electron beam current pulse amplitude was 5 A. The gas mixtures were used containing Xe (38-700 Torr) and CCl4 (0.03-0.3 Torr). The studies were performed within the wavelength range 200-1200 nm using a MAYA-2000Pro diffraction grating spectrometer and a RIGOL DS 5022 ME fast digital oscilloscope. The luminescence lifetimes of the excimer molecules XeCl* (band with λmax = 308 nm) and Xe2Cl* (band with λmax = 486 nm) were measured, as well as the constants of quenching by the components of the gas mixture for Xe2Cl* molecules. A model of plasma-chemical processes for dense Xe—CCl4 gas mixtures with a very low content of the CCl4 donor is proposed. It is shown that in such 'poor' mixtures Xe2Cl* molecules are mainly produced as a result of recombination of the Xe2+ and Cl- ions.

  4. Luminescence characteristics of Xe{sub 2}Cl excimer molecules under pumping the dense Xe-CCl{sub 4} gas mixtures with a pulsed electron beam

    Energy Technology Data Exchange (ETDEWEB)

    Mis' kevich, A I; Jinbo, Guo [National Research Nuclear University ' Moscow Engineering Physics Institute' , Moscow (Russian Federation)

    2013-05-31

    Temporal and spectral characteristics of the luminescence of dense Xe-CCl{sub 4} gas mixtures of different composition, excited by a 5-ns pulsed electron beam, were measured. The energy of the electrons amounted to 150 keV and the electron beam current pulse amplitude was 5 A. The gas mixtures were used containing Xe (38-700 Torr) and CCl{sub 4} (0.03-0.3 Torr). The studies were performed within the wavelength range 200-1200 nm using a MAYA-2000Pro diffraction grating spectrometer and a RIGOL DS 5022 ME fast digital oscilloscope. The luminescence lifetimes of the excimer molecules XeCl* (band with {lambda}{sub max} = 308 nm) and Xe{sub 2}Cl* (band with {lambda}{sub max} = 486 nm) were measured, as well as the constants of quenching by the components of the gas mixture for Xe{sub 2}Cl* molecules. A model of plasma-chemical processes for dense Xe-CCl{sub 4} gas mixtures with a very low content of the CCl{sub 4} donor is proposed. It is shown that in such 'poor' mixtures Xe{sub 2}Cl* molecules are mainly produced as a result of recombination of the Xe{sub 2}{sup +} and Cl{sup -} ions. (active media)

  5. Effect of temperature and discharge voltage on the properties of Co-doped ZnO thin films deposited by pulsed electron beam ablation

    Science.gov (United States)

    Ali, Asghar; Henda, Redhouane; Fagerberg, Ragnar

    2017-11-01

    Cobalt-doped ZnO (CZO) thin films have been deposited from CoxZn1-xO (x = 0.20) target on Si (100) substrate by pulsed electron beam ablation (PEBA). The effects of process temperature (350 °C-800 °C) and electron beam acceleration voltage (15 kV, 16 kV) on the deposited films have been assessed. The films have been prepared at constant beam pulse frequency (2 Hz) and Argon background pressure (∼3 mTorr). The structure and surface morphology of CZO films have been investigated by scanning electron microscopy (SEM) and atomic force microscopy (AFM). As per SEM data, the results show that the films consist of Co rich nano-sized globules (∼20 nm-300 nm). Energy dispersive x-ray (EDX) measurements reveal that Co content in the films seems to be unaffected by accelerating voltage while it increases with temperature in the range 350 °C-450 °C. At higher deposition temperatures (600 °C & 800 °C), the films exhibit faceted particles and are relatively rough. The films deposited at 800 °C consist of a predominantly Co phase. X-ray photoelectron spectroscopy (XPS) data confirm the presence of metallic cobalt in the films, whose content increases with temperature but is practically unaffected by beam voltage. X-ray diffraction (XRD) analysis confirms the presence of herxagonal close-packed (hcp) metallic cobalt in the films.

  6. Half-sandwich structure of cyclopentadienyl dialuminum [Al2(eta5-C5H5)] from pulsed-field ionization electron spectroscopy and ab initio calculations.

    Science.gov (United States)

    Lei, Yuxiu; Yang, Dong-Sheng

    2008-02-21

    Cyclopentadienyl dialuminum [Al2Cp, Cp = C5H5] was prepared in a pulsed laser ablation cluster beam source and identified with a time-of-flight photoionization mass spectrometer. The high-resolution electron spectrum of this complex was obtained using pulsed-field ionization zero electron kinetic energy (ZEKE) photoelectron spectroscopy. Three isomeric structures with two Al atoms residing on the same or opposite sites of the Cp plane were predicted by second-order Møller-Plesset perturbation theory. A half-sandwich structure with an aluminum dimer perpendicular to the Cp plane was identified by the experiment. The ground electronic states of the neutral and ionized species are 2A' ' in Cs symmetry and 1A1 in C5v symmetry, respectively. In both the neutral and ionic states, one of the Al2 atoms binds with five carbons, and the metal-ligand bonding consists of orbital and electrostatic contributions. Ionization of the 2A' ' neutral state enhances the metal-ligand bonding but weakens the metal-metal interaction.

  7. LASER EMISSIONS FROM CO2 VIBRATIONAL TRANSITIONS IN A LOW TEMPERATURE SUPERSONIC FLOW EXCITED BY A PULSED ELECTRON BEAM STABILIZED DISCHARGE

    OpenAIRE

    Fontaine, B.; Forestier, B.; Gross, P.; Koudriavtsev, E.

    1980-01-01

    High power long pulse infrared laser emission has been achieved on CO2 molecule with the high density and very low temperature supersonic flow-electron beam-stabilized discharge excitation device developped at I.M.F.M. ([MATH] [MATH] 2 amagats, T [MATH] 70 - 150 K). Laser emission at [MATH] = 10.6 µ has been achieved for a resonant cavity set at the discharge location and also 3 cm downstream of the discharge location. With Ar/CO2, Ar/CO2/H2, He/CO2, and He/CO2/N2 mixtures, lasing energy and ...

  8. A Q-band low noise GaAs pHEMT MMIC power amplifier for pulse electron spin resonance spectrometer.

    Science.gov (United States)

    Sitnikov, A; Kalabukhova, E; Oliynyk, V; Kolisnichenko, M

    2017-05-01

    We present the design and development of a single stage pulse power amplifier working in the frequency range 32-38 GHz based on a monolithic microwave integrated circuit (MMIC). We have designed the MMIC power amplifier by using the commercially available packaged GaAs pseudomorphic high electron mobility transistor. The circuit fabrication and assembly process includes the elaboration of the matching networks for the MMIC power amplifier and their assembling as well as the topology outline and fabrication of the printed circuit board of the waveguide-microstrip line transitions. At room ambient temperature, the measured peak output power from the prototype amplifier is 35.5 dBm for 16.6 dBm input driving power, corresponding to 19 dB gain. The measured rise/fall time of the output microwave signal modulated by a high-speed PIN diode was obtained as 5-6 ns at 20-250 ns pulse width with 100 kHz pulse repetition rate frequency.

  9. A Q-band low noise GaAs pHEMT MMIC power amplifier for pulse electron spin resonance spectrometer

    Science.gov (United States)

    Sitnikov, A.; Kalabukhova, E.; Oliynyk, V.; Kolisnichenko, M.

    2017-05-01

    We present the design and development of a single stage pulse power amplifier working in the frequency range 32-38 GHz based on a monolithic microwave integrated circuit (MMIC). We have designed the MMIC power amplifier by using the commercially available packaged GaAs pseudomorphic high electron mobility transistor. The circuit fabrication and assembly process includes the elaboration of the matching networks for the MMIC power amplifier and their assembling as well as the topology outline and fabrication of the printed circuit board of the waveguide-microstrip line transitions. At room ambient temperature, the measured peak output power from the prototype amplifier is 35.5 dBm for 16.6 dBm input driving power, corresponding to 19 dB gain. The measured rise/fall time of the output microwave signal modulated by a high-speed PIN diode was obtained as 5-6 ns at 20-250 ns pulse width with 100 kHz pulse repetition rate frequency.

  10. Generating high-brightness and coherent soft x-ray pulses in the water window with a seeded free-electron laser

    Directory of Open Access Journals (Sweden)

    Kaishang Zhou

    2017-01-01

    Full Text Available We propose a new scheme to generate high-brightness and temporal coherent soft x-ray radiation in a seeded free-electron laser. The proposed scheme is based on the coherent harmonic generation (CHG and superradiant principles. A CHG scheme is first used to generate a coherent signal at ultrahigh harmonics of the seed. This coherent signal is then amplified by a series of chicane-undulator modules via the fresh bunch and superradiant processes in the following radiator. Using a representative of a realistic set of parameters, three-dimensional simulations have been carried out and the simulations results demonstrated that 10 GW-level ultrashort (∼20  fs coherent radiation pulses in the water window can be achieved by using a 1.6 GeV electron beam based on the proposed technique.

  11. Publisher Correction: Nanoplasmonic electron acceleration by attosecond-controlled forward rescattering in silver clusters.

    Science.gov (United States)

    Passig, Johannes; Zherebtsov, Sergey; Irsig, Robert; Arbeiter, Mathias; Peltz, Christian; Göde, Sebastian; Skruszewicz, Slawomir; Meiwes-Broer, Karl-Heinz; Tiggesbäumker, Josef; Kling, Matthias F; Fennel, Thomas

    2018-02-07

    The original PDF version of this Article contained an error in Equation 1. The original HTML version of this Article contained errors in Equation 2 and Equation 4. These errors have now been corrected in both the PDF and the HTML versions of the Article.

  12. Attosecond nanotechnology: NEMS of energy storage and nanostructural transformations in materials

    Science.gov (United States)

    Beznosyuk, Sergey A.; Zhukovsky, Mark S.; Maslova, Olga A.

    2015-10-01

    The attosecond technology of the nanoelectromechanical system (NEMS) energy storage as active center fast transformation of nanostructures in materials is considered. The self-organizing relaxation of the NEMS active center containing nanocube of 256-atoms limited by planes (100) in the FCC lattice matrix of 4d-transition metals (Ru, Rh, Pd) is described by the quantum NEMS-kinetics (NK) method. Typical for these metals change of the NEMS active center physicochemical characteristics during the time of relaxation is presented. There are three types of intermediate quasistationary states of the NEMS active center. Their forms are plainly distinguishable. The full relaxed NEMS active centers (Ru256, Rh256, Pd256) accumulate next storage energies: ERu = 2.27 eV/at, ERh = 1.67 eV/at, EPd = 3.02 eV/at.

  13. Attosecond nanotechnology: NEMS of energy storage and nanostructural transformations in materials

    Energy Technology Data Exchange (ETDEWEB)

    Beznosyuk, Sergey A., E-mail: bsa1953@mail.ru; Maslova, Olga A., E-mail: maslova-o.a@mail.ru [Altai State University, Barnaul, 656049 (Russian Federation); Zhukovsky, Mark S., E-mail: zhukovsky@list.ru [Altai State Technical University, Barnaul, 656038 (Russian Federation)

    2015-10-27

    The attosecond technology of the nanoelectromechanical system (NEMS) energy storage as active center fast transformation of nanostructures in materials is considered. The self-organizing relaxation of the NEMS active center containing nanocube of 256-atoms limited by planes (100) in the FCC lattice matrix of 4d-transition metals (Ru, Rh, Pd) is described by the quantum NEMS-kinetics (NK) method. Typical for these metals change of the NEMS active center physicochemical characteristics during the time of relaxation is presented. There are three types of intermediate quasistationary states of the NEMS active center. Their forms are plainly distinguishable. The full relaxed NEMS active centers (Ru{sub 256}, Rh{sub 256}, Pd{sub 256}) accumulate next storage energies: E{sub Ru} = 2.27 eV/at, E{sub Rh} = 1.67 eV/at, E{sub Pd} = 3.02 eV/at.

  14. Tomographic reconstruction of circularly polarized high-harmonic fields: 3D attosecond metrology.

    Science.gov (United States)

    Chen, Cong; Tao, Zhensheng; Hernández-García, Carlos; Matyba, Piotr; Carr, Adra; Knut, Ronny; Kfir, Ofer; Zusin, Dimitry; Gentry, Christian; Grychtol, Patrik; Cohen, Oren; Plaja, Luis; Becker, Andreas; Jaron-Becker, Agnieszka; Kapteyn, Henry; Murnane, Margaret

    2016-02-01

    Bright, circularly polarized, extreme ultraviolet (EUV) and soft x-ray high-harmonic beams can now be produced using counter-rotating circularly polarized driving laser fields. Although the resulting circularly polarized harmonics consist of relatively simple pairs of peaks in the spectral domain, in the time domain, the field is predicted to emerge as a complex series of rotating linearly polarized bursts, varying rapidly in amplitude, frequency, and polarization. We extend attosecond metrology techniques to circularly polarized light by simultaneously irradiating a copper surface with circularly polarized high-harmonic and linearly polarized infrared laser fields. The resulting temporal modulation of the photoelectron spectra carries essential phase information about the EUV field. Utilizing the polarization selectivity of the solid surface and by rotating the circularly polarized EUV field in space, we fully retrieve the amplitude and phase of the circularly polarized harmonics, allowing us to reconstruct one of the most complex coherent light fields produced to date.

  15. Transverse Dynamics and Energy Tuning of Fast Electrons Generated in Sub-Relativistic Intensity Laser Pulse Interaction with Plasmas

    OpenAIRE

    Mori, M.; Kando, M.; Daito, I.; Kotaki, H.; Hayashi, Y.; Yamazaki, A.; Ogura, K.; Sagisaka, A.; Koga, J.; Nakajima, K.; Daido, H.; Bulanov, S. V.; Kimura, T.

    2006-01-01

    The regimes of quasi-mono-energetic electron beam generation were experimentally studied in the sub-relativistic intensity laser plasma interaction. The observed electron acceleration regime is unfolded with two-dimensional-particle-in-cell simulations of laser-wakefield generation in the self-modulation regime.

  16. Transverse dynamics and energy tuning of fast electrons generated in sub-relativistic intensity laser pulse interaction with plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Mori, M. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan)]. E-mail: mori.michiaki@jaea.go.jp; Kando, M. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan); Daito, I. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan); Kotaki, H. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan); Hayashi, Y. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan); Yamazaki, A. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan); Ogura, K. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan); Sagisaka, A. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan); Koga, J. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan); Nakajima, K. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan); Daido, H. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan); Bulanov, S.V.; Kimura, T. [Advanced Photon Research Center, Quantum Beam Science Directorate, Japan Atomic Energy Agency, Umemidai 8-1, Kizu, Kyoto 619-0215 (Japan)

    2006-07-31

    The regimes of quasi-monoenergetic electron beam generation were experimentally studied in the sub-relativistic intensity laser plasma interaction. The observed electron acceleration regime is unfolded with two-dimensional-particle-in-cell simulations of laser-wakefield generation in the self-modulation regime.

  17. Two-dimensional electron density measurement of pulsed positive primary streamer discharge in atmospheric-pressure air

    Science.gov (United States)

    Inada, Yuki; Aono, Kaiho; Ono, Ryo; Kumada, Akiko; Hidaka, Kunihiko; Maeyama, Mitsuaki

    2017-05-01

    Elucidating the electron density of streamer discharges propagating in atmospheric-pressure air is critical for achieving a systematic understanding of the production mechanisms of reactive species. Using Shack-Hartmann-type laser wavefront sensors with a temporal resolution of 2 ns, we carried out single-shot two-dimensional electron density measurements for positive primary streamers generated in a 13 mm air gap between pin-to-plate electrodes. The electron density over the positive primary streamers decayed from 1015 to {{10}14}\\text{c}{{\\text{m}}-3} during the propagation. The decay time constant of the electron density in the primary streamer channels was estimated to be  ˜2 ns. The distribution widths of the electron density were in good agreement with those of the light emission, typically ranging from 0.8 to 1.5 mm.

  18. Ultrafast Processes in Atoms and Molecules: Integrated treatment of electronic and nuclear motion in ultrashort XUV pulses

    Energy Technology Data Exchange (ETDEWEB)

    McCurdy, C. William [Univ. of California, Davis, CA (United States). Dept. of

    2017-12-14

    This project made use of Multiconfiguration Time-Dependent Hartree-Fock method developed earlier in the McCurdy group in a series of novel applications of the method to ultrafast spectroscopic processes. MCTDHF treats the dynamics of a molecule or atom under the influence of an external field in manner that has all electrons active. That property distinguishes this method from the more popular (and much less computationally demanding) approaches for treating the electron dynamics of atoms and molecules in fields, such as the time-dependent “Configuration Interaction Singles” approximation or approaches that limit the treatment to either one or two-electron models.

  19. Development of double-pulse lasers ablation system and electron paramagnetic resonance spectroscopy for direct spectral analysis of manganese doped PVA polymer

    Science.gov (United States)

    Khalil, A. A. I.; Morsy, M. A.; El-Deen, H. Z.

    2017-11-01

    Series of manganese-co-precipitated poly (vinyl alcohol) (PVA) polymer were quantitatively and qualitatively analyzed using laser ablation system (LAS) based on double-pulse laser induced breakdown spectroscopy (DP-LIBS) and electron paramagnetic resonance (EPR) spectroscopy. The collinear nanosecond laser beams of 266 and 1064 nm were optimized to focus on the surface of the PVA polymer target. Both laser beams were employed to estimate the natural properties of the excited Mn-PVA plasma, such as electron number density (Ne), electron temperature (Te), and Mn concentration. Individual transition lines of manganese (Mn), carbon (C), lithium (Li), hydrogen (H) and oxygen (O) atoms are identified based on the NIST spectral database. The results show better responses with DP-LIBS than the single-pulse laser induced breakdown spectroscopy (SP-LIBS). On the other hand, the EPR investigation shows characteristic broad peak of Mn-nano-particles (Mn-NPs) in the range of quantum dots of superparamagnetic materials. The line width (peak-to-peak, ΔHpp) and g-value of the observed Mn-EPR peak are ∼20 mT and 2.0046, respectively. The intensities of Mn-emission line at a wavelength 403.07 nm and the Mn-EPR absorption peak were used to accurate quantify the Mn-content in the polymer matrix. The results produce linear trends within the studied concentration range with regression coefficient (R2) value of ∼0.99, and limit of detection (LOD) of 0.026 mol.% and 0.016 mol.%, respectively. The LOD values are at a fold change of about -0.2 of the studied lowest mol.%. The proposed protocols of trace element detection are of significant advantage and can be applied to the other metal analysis.

  20. Selective excitation of a vibrational level within the electronic ground state of a polyatomic molecule with ultra pulses

    CSIR Research Space (South Africa)

    de Clercq, L

    2010-09-01

    Full Text Available Coherent control of the upper vibrational level populations in the electronic ground state of a polyatomic molecule was simulated. Results indicate that selective excitation of a specific upper state level is possible...