WorldWideScience

Sample records for atomic vapor laser

  1. A heated vapor cell unit for dichroic atomic vapor laser lock in atomic rubidium.

    Science.gov (United States)

    McCarron, Daniel J; Hughes, Ifan G; Tierney, Patrick; Cornish, Simon L

    2007-09-01

    The design and performance of a compact heated vapor cell unit for realizing a dichroic atomic vapor laser lock (DAVLL) for the D(2) transitions in atomic rubidium is described. A 5 cm long vapor cell is placed in a double-solenoid arrangement to produce the required magnetic field; the heat from the solenoid is used to increase the vapor pressure and correspondingly the DAVLL signal. We have characterized experimentally the dependence of important features of the DAVLL signal on magnetic field and cell temperature. For the weaker transitions both the amplitude and gradient of the signal are increased by an order of magnitude. PMID:17902946

  2. A heated vapor cell unit for dichroic atomic vapor laser lock in atomic rubidium

    International Nuclear Information System (INIS)

    The design and performance of a compact heated vapor cell unit for realizing a dichroic atomic vapor laser lock (DAVLL) for the D2 transitions in atomic rubidium is described. A 5 cm long vapor cell is placed in a double-solenoid arrangement to produce the required magnetic field; the heat from the solenoid is used to increase the vapor pressure and correspondingly the DAVLL signal. We have characterized experimentally the dependence of important features of the DAVLL signal on magnetic field and cell temperature. For the weaker transitions both the amplitude and gradient of the signal are increased by an order of magnitude

  3. [Atomic Vapor Laser Isotope Separation (AVLIS) program

    International Nuclear Information System (INIS)

    This report summarizes work performed for the Atomic Vapor Laser Isotope Separation (AVLIS) program from January through July, 1992. Each of the tasks assigned during this period is described, and results are presented. Section I details work on sensitivity matrices for the UDS relay telescope. These matrices show which combination of mirror motions may be performed in order to effect certain changes in beam parameters. In Section II, an analysis is given of transmission through a clipping aperture on the launch telescope deformable mirror. Observed large transmission losses could not be simulated in the analysis. An EXCEL spreadsheet program designed for in situ analysis of UDS optical systems is described in Section III. This spreadsheet permits analysis of changes in beam first-order characteristics due to changes in any optical system parameter, simple optimization to predict mirror motions needed to effect a combination of changes in beam parameters, and plotting of a variety of first-order data. Optical systems may be assembled directly from OSSD data. A CODE V nonsequential model of the UDS optical system is described in Section IV. This uses OSSD data to build the UDS model; mirror coordinates may thus be verified. Section V summarizes observations of relay telescope performance. Possible procedures which allow more accurate assessment of relay telescope performance are given

  4. Atomic vapor laser isotope separation using resonance ionization

    International Nuclear Information System (INIS)

    In June 1985, the Department of Energy announced the selection of atomic vapor laser isotope separation [AVLIS] as the technology to meet the United States' future need for enriched uranium. Resonance photoionization is the heart of the AVLIS process. The authors discuss those fundamental atomic parameters that are necessary for describing isotope-selective resonant multistep photoionization along with the measurement techniques employed. The methodology adopted is illustrated with examples of other elements that are under study in the program. (author)

  5. Lawrence Livermore National Laboratory's Atomic Vapor Laser Isotope Separation program: laser technology and demonstration facilities

    International Nuclear Information System (INIS)

    The Atomic Vapor Laser Isotope Separation (AVLIS) program at Lawrence Livermore National Laboratory (LLNL) is developing a large-scale process for photophysically enriching isotopes of several elements. The program now deploys plant prototypical hardware to demonstrate this enrichment process at full scale. The Laser Demonstration Facility, a fully integrated laser system has been constructed and when complete will produce more than 5000 W of tunable average power at a pulse repetition frequency >10 kHz. In AVLIS, an atomic vapor of mixed isotopes is irradiated with laser light precisely tuned to photoionize only desired isotopes. The resulting electrically charged photoions are deflected in an electric field to collector (or extractor) plates where they condense as enriched products. The AVLIS laser system consists of a series of high-average-power dye lasers optically pumped by an array of copper lasers. The dye lasers are used to do the three-step photoionization process. These lasers are well suited for the AVLIS process for both technical and economic reasons. They provide the precise narrowband (<100-MHz), short-pulse (<100-nsec), high-average-power, high-repetition-frequency laser light required by the atomic spectroscopy and vapor flow properties. Equally important, the capital and operating costs of this laser system in its present state of development are consistent with a commercially viable process deployment

  6. Some energy levels, which can be used in atomic vapor laser isotope separation

    International Nuclear Information System (INIS)

    In this study the bibliographical data concerning energy levels, isotope shifts and hyperfine splitting constants of the following elements were collected: Fe, Ca, Nd, Eu, Dy, La, Pb, Sm, Ba, Ti, Ta, Mg, V, Zr, Pu, Na, K, Li, Tc, Ni, Ag, Sn, Bk, Am, Np, Th. This Database is very useful for AVLIS and can help by choosing the equipment for atomic vapor laser isotope separation. Wavelength, waveform and bandwidth of the used laser are determined by this data. The properties of the vaporizer, separation chamber, and collection system are influenced by this data. This database is also necessary for calculations of the excitation selectivity. (author)

  7. Dichroic atomic vapor laser lock with multi-gigahertz stabilization range

    CERN Document Server

    Pustelny, S; Sholtes, T; Budker, D

    2015-01-01

    A dichroic atomic vapor laser lock (DAVLL) system exploiting buffer-gas-filled millimeter-scale vapor cells is presented. This system offers similar stability as achievable with bulk vapor cells, but has several important advantages. In addition to its compactness, it may provide continuous stabilization in a multi-gigahertz range around the optical transition. This range may be controlled either by changing the temperature of the vapor or by application of a buffer gas under an appropriate pressure. In particular, we show that the DAVLL system with a buffer-gas cell enables locking the laser frequency between two hyperfine components of the $^{85}$Rb ground state or as far as 16 GHz away from the closest optical transition.

  8. Dichroic atomic vapor laser lock with multi-gigahertz stabilization range

    Science.gov (United States)

    Pustelny, S.; Schultze, V.; Scholtes, T.; Budker, D.

    2016-06-01

    A dichroic atomic vapor laser lock (DAVLL) system exploiting buffer-gas-filled millimeter-scale vapor cells is presented. This system offers similar stability as achievable with conventional DAVLL system using bulk vapor cells, but has several important advantages. In addition to its compactness, it may provide continuous stabilization in a multi-gigahertz range around the optical transition. This range may be controlled either by changing the temperature of the vapor or by application of a buffer gas under an appropriate pressure. In particular, we experimentally demonstrate the ability of the system to lock the laser frequency between two hyperfine components of the 85Rb ground state or as far as 16 GHz away from the closest optical transition.

  9. Two-photon dichroic atomic vapor laser lock using electromagnetically induced transparency and absorption

    International Nuclear Information System (INIS)

    We demonstrate a technique to lock the frequency of a laser to a transition between two excited states in Rb vapor using a two-photon process in the presence of a weak magnetic field. We use a ladder configuration from specific hyperfine sublevels of the 5S1/2, 5P3/2, and 5D5/2 levels. This atomic configuration can show electromagnetically induced transparency and absorption processes. The error signal comes from the difference in the transparency or absorption felt by the two orthogonal polarizations of the probe beam. A simplified model is in good quantitative agreement with the observed signals for the experimental parameters. We have used this technique to lock the frequency of the laser up to 1.5 GHz off atomic resonance.

  10. Observation of picosecond superfluorescent pulses in rubidium atomic vapor pumped by 100-fs laser pulses

    International Nuclear Information System (INIS)

    We study the superfluorescence (SF) from a gas of rubidium atoms. The atoms of a dense vapor are excited to the 5D state from the 5S state by a two-photon process driven by 100-fs laser pulses. The atoms decay to the 6P state and then to the 5S state. The SF emission at 420 nm on the 6P-5S transition is recorded by a streak camera with picosecond time resolution. The time duration of the generated SF is tens of picoseconds, which is much shorter than the time scale of the usual relaxation processes, including spontaneous emission and atomic coherence dephasing. The dependence of the time delay between the reference input pulse and SF is measured as a function of laser power. The experimental data are described quantitatively by a simulation based on the semiclassical atom-field interaction theory. The observed change in scaling laws for the peak intensity and delay time can be elucidated by an SF theory in which the sample length is larger than the cooperation length.

  11. Study on laser atomic spectroscopy

    International Nuclear Information System (INIS)

    Electric discharge type atomic vaporizer is developed for the spectroscopic study on actinide elements. Laser induced fluorescence study on actinide elements is performed by using this high temperature type atomizer. For the effective photoionization of elements, copper vapor laser pumped dye laser and electron beam heating type atomic vaporizer are built and their characteristics are measured. In addition, resonance ionization mass spectroscopic analysis for lead sample as well as laser induced fluorescence study on uranium sample in solution phase is made. (Author)

  12. Self-generating magnetometer with laser pumping employment in “end resonance” wall coated vapor cell atomic clocks

    Science.gov (United States)

    Baranov, A. A.; Ermak, S. V.; Smolin, R. V.; Semenov, V. V.

    2016-06-01

    This paper presents the results of two double resonance signals correlation investigation. These signals were observed synchronously in optically oriented Rb87 vapors with laser pumping in a dual scheme: low frequency Mx-magnetometer and microwave frequency discriminator. Analytical studies of the scalar and vector light shift components contribution to the frequency instability of the end resonance microwave transitions are presented. An experimental demonstration of the light shift components mutual compensation in optically pumped Rb87 atoms was provided. The results were processed in terms of Allan variance, which demonstrated an effect of decreasing frequency variation at averaging times more than 100 s for a joint scheme of the end resonance microwave transition and selfgenerating (Mx) magnetometer.

  13. Atomic vapor laser isotope separation at Lawrence Livermore National Laboratory: a status report

    International Nuclear Information System (INIS)

    The field of laser induced chemistry began in earnest early in the 1970's with the initiation of major efforts in laser isotope separation (LIS) of uranium. Though many specialized, small-scale photochemical and diagnostic applications have been identified and evaluated experimentally, and continue to show promise, currently the only high payoff, large-scale applications remain LIS of special elements. Aspects of the physical scaling, technology status and economic basis of uranium LIS are examined with special emphasis on the effort at LLNL

  14. Detection of slow atoms confined in a Cesium vapor cell by spatially separated pump and probe laser beams

    CERN Document Server

    Todorov, Petko; Maurin, Isabelle; Saltiel, Solomon; Bloch, Daniel

    2013-01-01

    The velocity distribution of atoms in a thermal gas is usually described through a Maxwell-Boltzman distribution of energy, and assumes isotropy. As a consequence, the probability for an atom to leave the surface under an azimuth angle {\\theta} should evolve as cos {\\theta}, in spite of the fact that there is no microscopic basis to justify such a law. The contribution of atoms moving at a grazing incidence towards or from the surface, i.e. atoms with a small normal velocity, here called "slow" atoms, reveals essential in the development of spectroscopic methods probing a dilute atomic vapor in the vicinity of a surface, enabling a sub-Doppler resolution under a normal incidence irradiation. The probability for such "slow" atoms may be reduced by surface roughness and atom-surface interaction. Here, we describe a method to observe and to count these slow atoms relying on a mechanical discrimination, through spatially separated pump and probe beams. We also report on our experimental progresses toward such a g...

  15. Laser-induced transport effect and laser induced-line narrowing mechanism for laser excitation in 87Rb atomic vapors in a finite-size buffer-less cell

    International Nuclear Information System (INIS)

    Full text: Coherent population trapping (CPT) and double radio-optical resonance (DROR) are quantum nonlinear effects. Both these effects are the base for the creation of high precision magnetometers and atomic frequency standards. We study the influence of the laser induced transport (LIT) and the laser induced line narrowing (LILN) effects on the DROR and CPT resonance line shape for excitation in 87Rb atomic vapors in wall-coated and uncoated cell. We take into account both hyperfine and Zeeman structures of the ground and the excited states of 87Rb atoms as well as the probabilities of spontaneous transitions. We investigate the dependence of the resonance shape on the length of the cell, on the type of boundary conditions, on the polarization and intensity of laser and microwave fields, and on the laser line width ('narrow-band' and 'broad-band'). Laser induced transport in DROR: the first the LIT was predicted for three-level model. We show that the LIT takes place in buffer-less cell with real 87Rb atoms. The physical essence of the LIT effect is the caused by the Doppler effect velocity-selectivity of the interaction of 'narrow-band' laser field with atoms, resulting in Bennett dips and peaks in the velocity distribution of atoms in the ground state sublevels. Asymmetry of the two velocity distributions gives rise to the opposite-directed (along the laser propagation direction) fluxes of the atoms in the ground state sublevels. Therefore, a flux of the population inversion (or, equivalently, of the longitudinal magnetization) arises. This behavior one experimentally can obverse as the transmission peak in the centre of the DROR signal. LIT effect is most pronounced for 'narrow-band' laser pumping. Laser induced line narrowing in CPT resonance: the LILN of the CPT resonance realizes only in the case of excitation by 'narrow-band' laser. We established that for the LILN mechanism the parameters (the amplitude and width) of the CPT resonance excited on

  16. Study on laser atomic spectroscopy

    International Nuclear Information System (INIS)

    Laser atomic spectroscopic study on actinium element has been performed in many areas of spectroscopy. The study on characteristic of atomic vapor has been proceeded for copper atom and the spatial density distribution of copper vapor is measured. This experimental data has been compared with the theoretically calculated data. In spectroscopic experiment, the first and second excited states for actinium element are identified and the most efficient ionization scheme for actinium element is identified. In addition, the corrosion problem for filament material due to the heating of the actinium element has been studied. (Author)

  17. Environmental site description for a Uranium Atomic Vapor Laser Isotope Separation (U-AVLIS) production plant at the Paducah Gaseous Diffusion Plant site

    Energy Technology Data Exchange (ETDEWEB)

    Marmer, G.J.; Dunn, C.P.; Moeller, K.L.; Pfingston, J.M.; Policastro, A.J.; Yuen, C.R.; Cleland, J.H. (ed.)

    1991-09-01

    Uranium enrichment in the United States has utilized a diffusion process to preferentially enrich the U-235 isotope in the uranium product. The U-AVLIS process is based on electrostatic extraction of photoionized U-235 atoms from an atomic vapor stream created by electron-beam vaporization of uranium metal alloy. The U-235 atoms are ionized when precisely tuned laser light -- of appropriate power, spectral, and temporal characteristics -- illuminates the uranium vapor and selectively photoionizes the U-235 isotope. A programmatic document for use in screening DOE site to locate a U-AVLIS production plant was developed and implemented in two parts. The first part consisted of a series of screening analyses, based on exclusionary and other criteria, that identified a reasonable number of candidate sites. These sites were subjected to a more rigorous and detailed comparative analysis for the purpose of developing a short list of reasonable alternative sites for later environmental examination. This environmental site description (ESD) provides a detailed description of the PGDP site and vicinity suitable for use in an environmental impact statement (EIS). The report is based on existing literature, data collected at the site, and information collected by Argonne National Laboratory (ANL) staff during a site visit. 65 refs., 15 tabs.

  18. Environmental site description for a Uranium Atomic Vapor Laser Isotope Separation (U-AVLIS) production plant at the Paducah Gaseous Diffusion Plant site

    International Nuclear Information System (INIS)

    Uranium enrichment in the United States has utilized a diffusion process to preferentially enrich the U-235 isotope in the uranium product. The U-AVLIS process is based on electrostatic extraction of photoionized U-235 atoms from an atomic vapor stream created by electron-beam vaporization of uranium metal alloy. The U-235 atoms are ionized when precisely tuned laser light -- of appropriate power, spectral, and temporal characteristics -- illuminates the uranium vapor and selectively photoionizes the U-235 isotope. A programmatic document for use in screening DOE site to locate a U-AVLIS production plant was developed and implemented in two parts. The first part consisted of a series of screening analyses, based on exclusionary and other criteria, that identified a reasonable number of candidate sites. These sites were subjected to a more rigorous and detailed comparative analysis for the purpose of developing a short list of reasonable alternative sites for later environmental examination. This environmental site description (ESD) provides a detailed description of the PGDP site and vicinity suitable for use in an environmental impact statement (EIS). The report is based on existing literature, data collected at the site, and information collected by Argonne National Laboratory (ANL) staff during a site visit. 65 refs., 15 tabs

  19. A heated vapor cell unit for DAVLL in atomic rubidium

    CERN Document Server

    McCarron, Daniel J; Tierney, Patrick; Cornish, Simon L

    2007-01-01

    The design and performance of a compact heated vapor cell unit for realizing a dichroic atomic vapor laser lock (DAVLL) for the D2 transitions in atomic rubidium is described. A 5 cm-long vapor cell is placed in a double-solenoid arrangement to produce the required magnetic field; the heat from the solenoid is used to increase the vapor pressure and correspondingly the DAVLL signal. We have characterized experimentally the dependence of important features of the DAVLL signal on magnetic field and cell temperature. For the weaker transitions both the amplitude and gradient of the signal are increased by an order of magnitude.

  20. A heated vapor cell unit for DAVLL in atomic rubidium

    OpenAIRE

    McCarron, Daniel J.; Hughes, Ifan G; Tierney, Patrick; Cornish, Simon L.

    2007-01-01

    The design and performance of a compact heated vapor cell unit for realizing a dichroic atomic vapor laser lock (DAVLL) for the D2 transitions in atomic rubidium is described. A 5 cm-long vapor cell is placed in a double-solenoid arrangement to produce the required magnetic field; the heat from the solenoid is used to increase the vapor pressure and correspondingly the DAVLL signal. We have characterized experimentally the dependence of important features of the DAVLL signal on magnetic field...

  1. Atom laser divergence

    OpenAIRE

    Le Coq, Yann; Thywissen, Joseph H.; Rangwala, Sadiq A.; Gerbier, Fabrice; Richard, Simon; Delannoy, Guillaume; Bouyer, Philippe; Aspect, Alain

    2001-01-01

    We measure the angular divergence of a quasi-continuous, rf-outcoupled, free-falling atom laser as a function of the outcoupling frequency. The data is compared to a Gaussian-beam model of laser propagation that generalizes the standard formalism of photonic lasers. Our treatment includes diffraction, magnetic lensing, and interaction between the atom laser and the condensate. We find that the dominant source of divergence is the condensate-laser interaction.

  2. Environmental site description for a Uranium Atomic Vapor Laser Isotope Separation (U-AVLIS) production plant at the Oak Ridge Gaseous Diffusion Plant Site

    Energy Technology Data Exchange (ETDEWEB)

    1991-09-01

    In January 1990, the Secretary of Energy approved a plan for the demonstration and deployment of the Uranium Atomic Vapor Laser Isotope Separation (U-AVLIS) technology, with the near-term goal to provide the necessary information to make a deployment decision by November 1992. The U-AVLIS process is based on electrostatic extraction of photoionized U-235 atoms from an atomic vapor stream created by electron-beam vaporization of uranium metal alloy. A programmatic document for use in screening DOE sites to locate the U-AVLIS production plant was developed and implemented in two parts (Wolsko et al. 1991). The first part consisted of a series of screening analyses, based on exclusionary and other criteria, that identified a reasonable number of candidate sites. These sites were then subjected to a more rigorous and detailed comparative analysis for the purpose of developing a short list of reasonable alternative sites for later environmental examination. This environmental site description (ESD) provides a detailed description of the ORGDP site and vicinity suitable for use in an environmental impact statement (EIS). The report is based on existing literature, data collected at the site, and information collected by Argonne National Laboratory (ANL) staff during a site visit. The organization of the ESD is as follows. Topics addressed in Sec. 2 include a general site description and the disciplines of geology, water resources, biotic resources, air resources, noise, cultural resources, land use, socioeconomics, and waste management. Identification of any additional data that would be required for an EIS is presented in Sec. 3. Following the site description and additional data requirements, Sec. 4 provides a short, qualitative assessment of potential environmental issues. 37 refs., 20 figs., 18 tabs.

  3. Environmental site description for a Uranium Atomic Vapor Laser Isotope Separation (U-AVLIS) production plant at the Oak Ridge Gaseous Diffusion Plant Site

    International Nuclear Information System (INIS)

    In January 1990, the Secretary of Energy approved a plan for the demonstration and deployment of the Uranium Atomic Vapor Laser Isotope Separation (U-AVLIS) technology, with the near-term goal to provide the necessary information to make a deployment decision by November 1992. The U-AVLIS process is based on electrostatic extraction of photoionized U-235 atoms from an atomic vapor stream created by electron-beam vaporization of uranium metal alloy. A programmatic document for use in screening DOE sites to locate the U-AVLIS production plant was developed and implemented in two parts (Wolsko et al. 1991). The first part consisted of a series of screening analyses, based on exclusionary and other criteria, that identified a reasonable number of candidate sites. These sites were then subjected to a more rigorous and detailed comparative analysis for the purpose of developing a short list of reasonable alternative sites for later environmental examination. This environmental site description (ESD) provides a detailed description of the ORGDP site and vicinity suitable for use in an environmental impact statement (EIS). The report is based on existing literature, data collected at the site, and information collected by Argonne National Laboratory (ANL) staff during a site visit. The organization of the ESD is as follows. Topics addressed in Sec. 2 include a general site description and the disciplines of geology, water resources, biotic resources, air resources, noise, cultural resources, land use, socioeconomics, and waste management. Identification of any additional data that would be required for an EIS is presented in Sec. 3. Following the site description and additional data requirements, Sec. 4 provides a short, qualitative assessment of potential environmental issues. 37 refs., 20 figs., 18 tabs

  4. Low temperature operated copper vapor laser

    International Nuclear Information System (INIS)

    Experimental studies on newly developed copper vapor laser operated in hydrogen bromide gas under low temperature were successfully achieved using a conventional high temperature operated copper vapor laser tube. We present remarkable difference against conventional copper vapor laser in terms of the spatial and temporal features. This type of copper vapor laser is expected to have higher efficiency at high pulse repetition frequency and advantage in the features of laser pulse. (author)

  5. Metal atom oxidation laser

    International Nuclear Information System (INIS)

    A chemical laser which operates by formation of metal or carbon atoms and reaction of such atoms with a gaseous oxidizer in an optical resonant cavity is described. The lasing species are diatomic or polyatomic in nature and are readily produced by exchange or other abstraction reactions between the metal or carbon atoms and the oxidizer. The lasing molecules may be metal or carbon monohalides or monoxides

  6. Metal atom oxidation laser

    Science.gov (United States)

    Jensen, R.J.; Rice, W.W.; Beattie, W.H.

    1975-10-28

    A chemical laser which operates by formation of metal or carbon atoms and reaction of such atoms with a gaseous oxidizer in an optical resonant cavity is described. The lasing species are diatomic or polyatomic in nature and are readily produced by exchange or other abstraction reactions between the metal or carbon atoms and the oxidizer. The lasing molecules may be metal or carbon monohalides or monoxides. (auth)

  7. Analysis of organic vapors with laser induced breakdown spectroscopy

    International Nuclear Information System (INIS)

    In this paper, laser induced breakdown spectroscopy (LIBS) is utilized in the study of acetone, ethanol, methanol, cyclohexane, and nonane vapors. Carbon, hydrogen, oxygen, and nitrogen atomic emission spectra have been recorded following laser-induced breakdown of the organic vapors that are mixed with air inside a quartz chamber at atmospheric pressure. The plasma is generated with focused, Q-switched Nd:YAG radiation at the wavelength of 1064 nm. The effects of ignition and vapor pressure are discussed in view of the appearance of the emission spectra. The recorded spectra are proportional to the vapor pressure in air. The hydrogen and oxygen contributions diminish gradually with consecutive laser-plasma events without gas flow. The results show that LIBS can be used to characterize organic vapor

  8. Analysis of organic vapors with laser induced breakdown spectroscopy

    Science.gov (United States)

    Nozari, Hadi; Rezaei, Fatemeh; Tavassoli, Seyed Hassan

    2015-09-01

    In this paper, laser induced breakdown spectroscopy (LIBS) is utilized in the study of acetone, ethanol, methanol, cyclohexane, and nonane vapors. Carbon, hydrogen, oxygen, and nitrogen atomic emission spectra have been recorded following laser-induced breakdown of the organic vapors that are mixed with air inside a quartz chamber at atmospheric pressure. The plasma is generated with focused, Q-switched Nd:YAG radiation at the wavelength of 1064 nm. The effects of ignition and vapor pressure are discussed in view of the appearance of the emission spectra. The recorded spectra are proportional to the vapor pressure in air. The hydrogen and oxygen contributions diminish gradually with consecutive laser-plasma events without gas flow. The results show that LIBS can be used to characterize organic vapor.

  9. Analysis of organic vapors with laser induced breakdown spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Nozari, Hadi; Tavassoli, Seyed Hassan [Laser and Plasma Research Institute, Shahid Beheshti University, G. C, 1983963113 Evin, Tehran (Iran, Islamic Republic of); Rezaei, Fatemeh, E-mail: fatemehrezaei@kntu.ac.ir [Department of Physics, K. N. Toosi University of Technology, 15875-4416 Shariati, Tehran (Iran, Islamic Republic of)

    2015-09-15

    In this paper, laser induced breakdown spectroscopy (LIBS) is utilized in the study of acetone, ethanol, methanol, cyclohexane, and nonane vapors. Carbon, hydrogen, oxygen, and nitrogen atomic emission spectra have been recorded following laser-induced breakdown of the organic vapors that are mixed with air inside a quartz chamber at atmospheric pressure. The plasma is generated with focused, Q-switched Nd:YAG radiation at the wavelength of 1064 nm. The effects of ignition and vapor pressure are discussed in view of the appearance of the emission spectra. The recorded spectra are proportional to the vapor pressure in air. The hydrogen and oxygen contributions diminish gradually with consecutive laser-plasma events without gas flow. The results show that LIBS can be used to characterize organic vapor.

  10. Atomic vapor spectroscopy in integrated photonic structures

    CERN Document Server

    Ritter, Ralf; Pernice, Wolfram; Kübler, Harald; Pfau, Tilman; Löw, Robert

    2015-01-01

    We investigate an integrated optical chip immersed in atomic vapor providing several waveguide geometries for spectroscopy applications. The narrow-band transmission through a silicon nitride waveguide and interferometer is altered when the guided light is coupled to a vapor of rubidium atoms via the evanescent tail of the waveguide mode. We use grating couplers to couple between the waveguide mode and the radiating wave, which allow for addressing arbitrary coupling positions on the chip surface. The evanescent atom-light interaction can be numerically simulated and shows excellent agreement with our experimental data. This work demonstrates a next step towards miniaturization and integration of alkali atom spectroscopy and provides a platform for further fundamental studies of complex waveguide structures.

  11. Atomic vapor spectroscopy in integrated photonic structures

    Energy Technology Data Exchange (ETDEWEB)

    Ritter, Ralf; Kübler, Harald; Pfau, Tilman; Löw, Robert, E-mail: r.loew@physik.uni-stuttgart.de [5. Physikalisches Institut and Center for Integrated Quantum Science and Technology, Universität Stuttgart, Pfaffenwaldring 57, 70550 Stuttgart (Germany); Gruhler, Nico; Pernice, Wolfram [Institute of Nanotechnology, Karlsruhe Institute of Technology, 76344 Eggenstein-Leopoldshafen (Germany)

    2015-07-27

    We investigate an integrated optical chip immersed in atomic vapor providing several waveguide geometries for spectroscopy applications. The narrow-band transmission through a silicon nitride waveguide and interferometer is altered when the guided light is coupled to a vapor of rubidium atoms via the evanescent tail of the waveguide mode. We use grating couplers to couple between the waveguide mode and the radiating wave, which allow for addressing arbitrary coupling positions on the chip surface. The evanescent atom-light interaction can be numerically simulated and shows excellent agreement with our experimental data. This work demonstrates a next step towards miniaturization and integration of alkali atom spectroscopy and provides a platform for further fundamental studies of complex waveguide structures.

  12. Atomic iodine laser

    International Nuclear Information System (INIS)

    The atomic iodine photodissociation laser has been under intensive study for a number of years. The physics associated with this system is now well understood and it is possible to produce a 0.1 nsec (or longer) near-diffraction-limited laser pulse which can be amplified with negligible temporal distortion and little spatial deformation. The output of either a saturated or unsaturated amplifier consists of a high-fidelity near-diffraction-limited, energetic laser pulse. The report is divided into three chapters. Chapter 1 is a survey of the important areas affecting efficient laser operation and summarizes the findings of Chap. 2. Chapter 2 presents detailed discussions and evaluations pertinent to pumps, chemical regeneration, and other elements in the overall laser system. Chapter 3 briefly discusses those areas that require further work and the nature of the work required to complete the full-scale evaluation of the applicability of the iodine photodissociation laser to the inertial confinement program

  13. Atomic iodine laser

    Energy Technology Data Exchange (ETDEWEB)

    Fisk, G.A.; Gusinow, M.A.; Hays, A.K.; Padrick, T.D.; Palmer, R.E.; Rice, J.K.; Truby, F.K.; Riley, M.E.

    1978-05-01

    The atomic iodine photodissociation laser has been under intensive study for a number of years. The physics associated with this system is now well understood and it is possible to produce a 0.1 nsec (or longer) near-diffraction-limited laser pulse which can be amplified with negligible temporal distortion and little spatial deformation. The output of either a saturated or unsaturated amplifier consists of a high-fidelity near-diffraction-limited, energetic laser pulse. The report is divided into three chapters. Chapter 1 is a survey of the important areas affecting efficient laser operation and summarizes the findings of Chap. 2. Chapter 2 presents detailed discussions and evaluations pertinent to pumps, chemical regeneration, and other elements in the overall laser system. Chapter 3 briefly discusses those areas that require further work and the nature of the work required to complete the full-scale evaluation of the applicability of the iodine photodissociation laser to the inertial confinement program.

  14. Optical Multidimensional Spectroscopy of Atomic Vapor

    Directory of Open Access Journals (Sweden)

    Siemens Mark E.

    2013-03-01

    Full Text Available Optical single- and double-quantum three-dimensional Fourier-transform spectra are obtained for atomic vapors. We show that three-dimensional spectra can be used to identify the Hamiltonian of complex systems and to reveal the nature of many-body interactions.

  15. Analysis of laser beam propagation effects in atomic laser isotope separation

    International Nuclear Information System (INIS)

    In the atomic laser isotope separation process, the laser beams propagate through the atomic vapor over a long distance. It has been shown that the laser-atom interactions significantly modify the laser pulse shape and propagation velocity, resulting in degradation of the isotope separation efficiency. These propagation effects have been analyzed quantitatively, and a simple scaling formula has been derived to estimate the necessary laser energy for such optically thick atomic vapor. The optimum conditions of incident laser pulse have also been discussed. (author)

  16. Guided Quasicontinuous Atom Laser

    OpenAIRE

    Guerin, William; Riou, Jean-Félix; Gaebler, John,; Josse, Vincent; Bouyer, Philippe; Aspect, Alain

    2006-01-01

    version published in Phys. Rev. Lett. 97, 200402 (2006) International audience We report the first realization of a guided quasicontinuous atom laser by rf outcoupling a Bose-Einstein condensate from a hybrid optomagnetic trap into a horizontal atomic waveguide. This configuration allows us to cancel the acceleration due to gravity and keep the de Broglie wavelength constant at 0.5 µm during 0.1 s of propagation. We also show that our configuration, equivalent to pigtailing an optical f...

  17. Environmental site description for a Uranium Atomic Vapor Laser Isotope Separation (U-AVLIS) production plant at the Portsmouth Gaseous Diffusion Plant site

    International Nuclear Information System (INIS)

    Uranium enrichment in the United States has utilized a diffusion process to preferentially enrich the U-235 isotope in the uranium product. In the 1970s, the US Department of Energy (DOE) began investigating more efficient and cost-effective enrichment technologies. In January 1990, the Secretary of Energy approved a plan for the demonstration and deployment of the Uranium Atomic Vapor Laser isotope Separation (U-AVLIS) technology with the near-term goal to provide the necessary information to make a deployment decision by November 1992. Initial facility operation is anticipated for 1999. A programmatic document for use in screening DOE sites to locate a U-AVLIS production plant was developed and implemented in two parts. The first part consisted of a series of screening analyses, based on exclusionary and other criteria, that identified a reasonable number of candidate sites. The final evaluation, which included sensitivity studies, identified the Oak Ridge Gaseous Diffusion Plant (ORGDP) site, the Paducah Gaseous Diffusion Plant (PGDP) site, and the Portsmouth Gaseous Diffusion Plant (PORTS) site as having significant advantages over the other sites considered. This environmental site description (ESD) provides a detailed description of the PORTS site and vicinity suitable for use in an environmental impact statement (EIS). This report is based on existing literature, data collected at the site, and information collected by Argonne National Laboratory (ANL) staff during site visits. The organization of the ESD is as follows. Topics addressed in Sec. 2 include a general site description and the disciplines of geology, water resources, biotic resources, air resources, noise, cultural resources, land use. Socioeconomics, and waste management. Identification of any additional data that would be required for an EIS is presented in Sec. 3

  18. Environmental site description for a Uranium Atomic Vapor Laser Isotope Separation (U-AVLIS) production plant at the Portsmouth Gaseous Diffusion Plant site

    Energy Technology Data Exchange (ETDEWEB)

    Marmer, G.J.; Dunn, C.P.; Filley, T.H.; Moeller, K.L.; Pfingston, J.M.; Policastro, A.J.; Cleland, J.H.

    1991-09-01

    Uranium enrichment in the United States has utilized a diffusion process to preferentially enrich the U-235 isotope in the uranium product. In the 1970s, the US Department of Energy (DOE) began investigating more efficient and cost-effective enrichment technologies. In January 1990, the Secretary of Energy approved a plan for the demonstration and deployment of the Uranium Atomic Vapor Laser isotope Separation (U-AVLIS) technology with the near-term goal to provide the necessary information to make a deployment decision by November 1992. Initial facility operation is anticipated for 1999. A programmatic document for use in screening DOE sites to locate a U-AVLIS production plant was developed and implemented in two parts. The first part consisted of a series of screening analyses, based on exclusionary and other criteria, that identified a reasonable number of candidate sites. The final evaluation, which included sensitivity studies, identified the Oak Ridge Gaseous Diffusion Plant (ORGDP) site, the Paducah Gaseous Diffusion Plant (PGDP) site, and the Portsmouth Gaseous Diffusion Plant (PORTS) site as having significant advantages over the other sites considered. This environmental site description (ESD) provides a detailed description of the PORTS site and vicinity suitable for use in an environmental impact statement (EIS). This report is based on existing literature, data collected at the site, and information collected by Argonne National Laboratory (ANL) staff during site visits. The organization of the ESD is as follows. Topics addressed in Sec. 2 include a general site description and the disciplines of geology, water resources, biotic resources, air resources, noise, cultural resources, land use. Socioeconomics, and waste management. Identification of any additional data that would be required for an EIS is presented in Sec. 3.

  19. Copper vapor laser system development

    International Nuclear Information System (INIS)

    High-power, high-quality, and long-life copper vapor laser (CVL) system has been developed and operated. The system is composed of a small sized CVL oscillator with high beam quality, several high-power CVL amplifiers and related sub-systems such as special resonator optics, beam shaping and propagating optics, and pulse timing controller. Further developments of high-power amplifiers are being conducted for the next R and D targets. In our latest tests, the maximum output power of 480W has been achieved by optimizing discharge circuit conditions. Major-components life-time of more than 2000 hours has been also ensured in long-term CVL amplifier operation tests. Accumulated operation time of more than 700 hours has been achieved without refilling copper source or any maintenance. (author)

  20. Dispersive radio frequency electrometry using Rydberg atoms in a prism-shaped atomic vapor cell

    Science.gov (United States)

    Fan, H. Q.; Kumar, S.; Kübler, H.; Shaffer, J. P.

    2016-05-01

    We introduce a method to measure radio frequency (RF) electric fields (E-fields) using atoms contained in a prism-shaped vapor cell. The method utilizes the concept of electromagnetically induced transparency with Rydberg atoms. The RF E-field induces changes in the index of refraction of the vapor resulting in deflection of the probe laser beam as it passes through the prism-shaped vapor cell. We measured a minimum RF E-field of 8.25 μ {{Vcm}}-1 with a sensitivity of ∼ 46.5 μ {{Vcm}}-1 {{Hz}}-1/2. The experimental results agree with a numerical model that includes dephasing effects. We discuss possible improvements to obtain higher sensitivity for RF E-field measurements.

  1. Investigations on atomic-vapor-filter high-spectral-resolution lidar for temperature measurements

    Science.gov (United States)

    Voss, E.; Weitkamp, C.

    1992-01-01

    The temperature measurement by the analysis of Rayleigh scattered laser radiation with atomic vapor filters is investigated in both theory and laboratory experiments. Synthetic air is irradiated with a cw dye laser at 283 nano-meters, and the backscattered spectrum is analyzed with two lead vapor cells in one oven. Temperature measurements are carried out, and the effect of different parameters on the accuracy is investigated. Important aspects for the realization of a lidar are given.

  2. Low temperature laser physical vapor deposition of multilayered thin films

    International Nuclear Information System (INIS)

    The authors have investigated the formation of various multilayer thin films by the laser physical vapor deposition technique. A multi stage target holder was constructed to perform all process steps in-situ; target/substrate cleaning, deposition, and annealing. The laser physical vapor deposition technique offers many advantages over conventional physical vapor techniques, such as, lower substrate temperature, microstructural control, and very low contamination levels. Film thickness can be controlled from near atomic to micron dimensions. A layer-by-layer (two dimensional) growth can be achieved, resulting in nonequilibrium structures. The films were analyzed using cross-section and high resolution transmission electron microscopy (TEM). The significant reduction in substrate temperature for the formation of high quality multilayer and epitaxial films opens up many new areas of applications requiring reduced thermal-budget processing. The authors present results of sequential deposition of multilayered thin films of carbon and tungsten, titanium nitride and carbide, and high Tc superconductor compounds

  3. Photo- and chemo ionization processes in the saturated rubidium vapors at resonant-excited atomic transition

    International Nuclear Information System (INIS)

    The mutual competition of the two-photon, associative, and penning ionization of the resonant-excited rubidium atoms in a dye-laser field has been investigated. For each ionization channel the ranges of laser intensities and rubidium vapor pressure are determined within the limits of that its contribution is predominant. On the basis of the data obtained the cross section of photo- and collision ionization processes of excited atoms are determined. (author)

  4. Metal vapor lasers with increased reliability

    Science.gov (United States)

    Soldatov, A. N.; Sabotinov, N. V.; Polunin, Yu. P.; Shumeiko, A. S.; Kostadinov, I. K.; Vasilieva, A. V.; Reimer, I. V.

    2015-12-01

    Results of investigation and development of an excitation pulse generator with magnetic pulse compression by saturation chokes for pumping of active media of CuBr, Sr, and Ca vapor lasers are presented. A high-power IGBT transistor is used as a commutator. The generator can operate at excitation pulse repetition frequencies up to 20 kHz. The total average power for all laser lines of the CuBr laser pumped by this generator is ~6.0 W; it is ~1.3-1.7 W for the Sr and Ca lasers.

  5. New Medical Applications Of Metal Vapor Lasers

    Science.gov (United States)

    Anderson, Robert S.; McIntosh, Alexander I.

    1989-06-01

    The first medical application for metal vapor lasers has been granted marketing approval by the FDA. This represents a major milestone for this technology. Metalaser Technologies recently received this approval for its Vasculase unit in the treatment of vascular lesions such as port wine stains, facial telangiectasia and strawberry hemangiomas.

  6. Copper vapor laser place in the laser isotope separation program

    OpenAIRE

    Lemaire, P.; Maury, J.

    1994-01-01

    The French uranium enrichment program, SILVA (Séparation Isotopique par Laser de la Vapeur Atomique d'uranium), has chosen yet the Copper Vapor Laser (CVL) for dye laser pumping. CVL is the most efficient laser in the visible, for pulsed operation, and with a high repetition rate. Over 400W of average optical power is achived from one unit ; work is done under CEA/CILAS contract. A 120W laser, the ICL 100 is available on the market from CEA/CILAS. MTBF over 1000 h is specified. In MOPA (Maste...

  7. Single molecule DNA detection with an atomic vapor notch filter

    Energy Technology Data Exchange (ETDEWEB)

    Uhland, Denis; Rendler, Torsten; Widmann, Matthias; Lee, Sang-Yun [University of Stuttgart and Stuttgart Research Center of Photonic Engineering (SCoPE) and IQST, 3rd Physics Institute, Stuttgart (Germany); Wrachtrup, Joerg; Gerhardt, Ilja [University of Stuttgart and Stuttgart Research Center of Photonic Engineering (SCoPE) and IQST, 3rd Physics Institute, Stuttgart (Germany); Max Planck Institute for Solid State Research, Stuttgart (Germany)

    2015-12-01

    The detection of single molecules has facilitated many advances in life- and material-science. Commonly the fluorescence of dye molecules is detected, which are attached to a non-fluorescent structure under study. For fluorescence microscopy one desires to maximize the detection efficiency together with an efficient suppression of undesired laser leakage. Here we present the use of the narrow-band filtering properties of hot atomic sodium vapor to selectively filter the excitation light from the red-shifted fluorescence of dye labeled single-stranded DNA molecules. A statistical analysis proves an enhancement in detection efficiency of more than 15% in a confocal and in a wide-field configuration. (orig.)

  8. Studies on laser atomic spectroscopy

    International Nuclear Information System (INIS)

    Laser atomic spectroscopy is studied both theoretically and experimentally. For Na-like ions, possible electric dipole, quadrupole and magnetic dipole transitions between atomic levels below 4f doublet F (J=7/2) state are investigated, using the recently developed computer programs - MCDF, MJE and MULTPOL. Line strength, oscillator strength and transition probability are calculated. A preliminary results for Hg-RIS experiment are also presented. Q-switched Nd:YAG laser, high power dye laser, vacuum system, ionization cell and ion measuring system are constructed, and their characteristics are examined. (Author)

  9. Investigation of odd-order nonlinear susceptibilities in atomic vapors

    Energy Technology Data Exchange (ETDEWEB)

    Yan, Yaqi [Key Laboratory for Physical Electronics and Devices of the Ministry of Education, Xi’an Jiaotong University, Xi’an 710049 (China); Shaanxi Key Laboratory of Information Photonic Technique, Xi’an Jiaotong University, Xi’an 710049 (China); Teaching and Research Section of Maths and Physics, Guangzhou Commanding Academy of Chinese People’s Armed Police Force, Guangzhou, 510440 (China); Wu, Zhenkun; Si, Jinhai; Yan, Lihe; Zhang, Yiqi; Yuan, Chenzhi; Sun, Jia [Key Laboratory for Physical Electronics and Devices of the Ministry of Education, Xi’an Jiaotong University, Xi’an 710049 (China); Shaanxi Key Laboratory of Information Photonic Technique, Xi’an Jiaotong University, Xi’an 710049 (China); Zhang, Yanpeng, E-mail: ypzhang@mail.xjtu.edu.cn [Key Laboratory for Physical Electronics and Devices of the Ministry of Education, Xi’an Jiaotong University, Xi’an 710049 (China); Shaanxi Key Laboratory of Information Photonic Technique, Xi’an Jiaotong University, Xi’an 710049 (China)

    2013-06-15

    We theoretically deduce the macroscopic symmetry constraints for arbitrary odd-order nonlinear susceptibilities in homogeneous media including atomic vapors for the first time. After theoretically calculating the expressions using a semiclassical method, we demonstrate that the expressions for third- and fifth-order nonlinear susceptibilities for undressed and dressed four- and six-wave mixing (FWM and SWM) in atomic vapors satisfy the macroscopic symmetry constraints. We experimentally demonstrate consistence between the macroscopic symmetry constraints and the semiclassical expressions for atomic vapors by observing polarization control of FWM and SWM processes. The experimental results are in reasonable agreement with our theoretical calculations. -- Highlights: •The macroscopic symmetry constraints are deduced for homogeneous media including atomic vapors. •We demonstrate that odd-order nonlinear susceptibilities satisfy the constraints. •We experimentally demonstrate the deduction in part.

  10. Dual-Beam Atom Laser Driven by Spinor Dynamics

    Science.gov (United States)

    Thompson, Robert; Lundblad, Nathan; Maleki, Lute; Aveline, David

    2007-01-01

    An atom laser now undergoing development simultaneously generates two pulsed beams of correlated Rb-87 atoms. (An atom laser is a source of atoms in beams characterized by coherent matter waves, analogous to a conventional laser, which is a source of coherent light waves.) The pumping mechanism of this atom laser is based on spinor dynamics in a Bose-Einstein condensate. By virtue of the angular-momentum conserving collisions that generate the two beams, the number of atoms in one beam is correlated with the number of atoms in the other beam. Such correlations are intimately linked to entanglement and squeezing in atomic ensembles, and atom lasers like this one could be used in exploring related aspects of Bose-Einstein condensates, and as components of future sensors relying on atom interferometry. In this atom-laser apparatus, a Bose-Einstein condensate of about 2 x 10(exp 6) Rb-87 atoms at a temperature of about 120 micro-K is first formed through all-optical means in a relatively weak singlebeam running-wave dipole trap that has been formed by focusing of a CO2-laser beam. By a technique that is established in the art, the trap is loaded from an ultrahigh-vacuum magnetooptical trap that is, itself, loaded via a cold atomic beam from an upstream two-dimensional magneto-optical trap that resides in a rubidium-vapor cell that is differentially pumped from an adjoining vacuum chamber, wherein are performed scientific observations of the beams ultimately generated by the atom laser.

  11. High resolution field imaging with atomic vapor cells

    OpenAIRE

    Horsley, Andrew

    2015-01-01

    In this thesis, I report on the development of imaging techniques in atomic vapor cells. This is a relatively unexplored area, despite the ubiquitous use of imaging in experiments with ultracold atoms. Our main focus is in high resolution imaging of microwave near fields, for which there is currently no satisfactory established technique. We detect microwave fields through Rabi oscillations driven by the microwave on atomic hyperfine transitions. The technique can be easily modified to also i...

  12. Laser spectroscopy of sputtered atoms

    International Nuclear Information System (INIS)

    The use of laser radiation to study the sputtering process is of relatively recent origin. Much has been learned from this work about the basic physics of the sputtering process itself through measurements of velocity and excited state distributions of sputtered atoms and the effects of adsorbates on substrate sputtering yields. Furthermore, the identification, characterization, and sensitive detection of sputtered atoms by laser spectroscopy has led to the development of in situ diagnostics for impurity fluxes in the plasma edge regions of tokamaks and of ultrasensitive methods (ppB Fe in Si) for surface analysis with ultralow (picocoulomb) ion fluences. The techniques involved in this work, laser fluorescence and multiphoton resonance ionization spectroscopy, will be described and illustrations given of results achieved up to now. 55 refs., 5 figs., 1 tab

  13. Femtosecond laser fluorescence and propagation in very dense potassium vapor.

    Science.gov (United States)

    Makdisi, Y; Kokaj, J; Afrousheh, K; Nair, R; Mathew, J; Pichler, G

    2013-12-16

    Femtosecond (fs) laser propagation and fluorescence of dense potassium vapor was studied, and the spectral region around the first and the second doublets of the principal series lines of potassium atoms was investigated. In our search we did not observe the conical emission in the far field, although it was previously observed in the case of rubidium. We discuss the possible reason of this unexpected result. The fluorescence spectrum revealed Rb impurity resonance lines in emission due to the collisional redistribution from the K(4p) levels into the Rb(5p) levels. In the forward propagation of 400 nm femtosecond light we observed the molecular band red shifted from potassium second doublet. However, no molecular spectrum was observed when the mode-locked fs laser light was discretely tuned within the wings of the first resonance lines, at 770 nm. PMID:24514609

  14. Radio-frequency Electrometry Using Rydberg Atoms in Vapor Cells: Towards the Shot Noise Limit

    Science.gov (United States)

    Kumar, Santosh; Fan, Haoquan; Jahangiri, Akbar; Kuebler, Harald; Shaffer, James P.; 5. Physikalisches Institut, Universitat Stuttgart, Germany Collaboration

    2016-05-01

    Rydberg atoms are a promising candidate for radio frequency (RF) electric field sensing. Our method uses electromagnetically induced transparency with Rydberg atoms in vapor cells to read out the effect that the RF electric field has on the Rydberg atoms. The method has the potential for high sensitivity (pV cm-1 Hz- 1 / 2) and can be self-calibrated. Some of the main factors limiting the sensitivity of RF electric field sensing from reaching the shot noise limit are the residual Doppler effect and the sensitivity of the optical read-out using the probe laser. We present progress on overcoming the residual Doppler effect by using a new multi-photon scheme and reaching the shot noise detection limit using frequency modulated spectroscopy. Our experiments also show promise for studying quantum optical effects such as superradiance in vapor cells using Rydberg atoms. This work is supported by DARPA, ARO, and NRO.

  15. Electrons and atoms in intense laser fields

    International Nuclear Information System (INIS)

    Several non-linear effects that show up when electrons and atoms interact with strong laser fields are considered. Thomson scattering, electron potential scattering in the presence of a laser beam, atomic ionization by strong laser fields, the refraction of electrons by laser beams and the Kapitza-Dirac effect are discussed. (Author)

  16. Focusing Light Beams To Improve Atomic-Vapor Optical Buffers

    Science.gov (United States)

    Strekalov, Dmitry; Matsko, Andrey; Savchenkov, Anatoliy

    2010-01-01

    Specially designed focusing of light beams has been proposed as a means of improving the performances of optical buffers based on cells containing hot atomic vapors (e.g., rubidium vapor). There is also a companion proposal to improve performance by use of incoherent optical pumping under suitable conditions. Regarding the proposal to use focusing: The utility of atomic-vapor optical buffers as optical storage and processing devices has been severely limited by nonuniform spatial distributions of intensity in optical beams, arising from absorption of the beams as they propagate in atomic-vapor cells. Such nonuniformity makes it impossible to optimize the physical conditions throughout a cell, thereby making it impossible to optimize the performance of the cell as an optical buffer. In practical terms simplified for the sake of brevity, "to optimize" as used here means to design the cell so as to maximize the group delay of an optical pulse while keeping the absorption and distortion of the pulse reasonably small. Regarding the proposal to use incoherent optical pumping: For reasons too complex to describe here, residual absorption of light is one of the main impediments to achievement of desirably long group delays in hot atomic vapors. The present proposal is directed toward suppressing residual absorption of light. The idea of improving the performance of slow-light optical buffers by use of incoherent pumping overlaps somewhat with the basic idea of Raman-based slow-light systems. However, prior studies of those systems did not quantitatively answer the question of whether the performance of an atomic vapor or other medium that exhibits electromagnetically induced transparency (EIT) with Raman gain is superior to that of a medium that exhibits EIT without Raman gain.

  17. Atom Skimmers and Atom Lasers Utilizing Them

    Science.gov (United States)

    Hulet, Randall; Tollett, Jeff; Franke, Kurt; Moss, Steve; Sackett, Charles; Gerton, Jordan; Ghaffari, Bita; McAlexander, W.; Strecker, K.; Homan, D.

    2005-01-01

    Atom skimmers are devices that act as low-pass velocity filters for atoms in thermal atomic beams. An atom skimmer operating in conjunction with a suitable thermal atomic-beam source (e.g., an oven in which cesium is heated) can serve as a source of slow atoms for a magneto-optical trap or other apparatus in an atomic-physics experiment. Phenomena that are studied in such apparatuses include Bose-Einstein condensation of atomic gases, spectra of trapped atoms, and collisions of slowly moving atoms. An atom skimmer includes a curved, low-thermal-conduction tube that leads from the outlet of a thermal atomic-beam source to the inlet of a magneto-optical trap or other device in which the selected low-velocity atoms are to be used. Permanent rare-earth magnets are placed around the tube in a yoke of high-magnetic-permeability material to establish a quadrupole or octupole magnetic field leading from the source to the trap. The atoms are attracted to the locus of minimum magnetic-field intensity in the middle of the tube, and the gradient of the magnetic field provides centripetal force that guides the atoms around the curve along the axis of the tube. The threshold velocity for guiding is dictated by the gradient of the magnetic field and the radius of curvature of the tube. Atoms moving at lesser velocities are successfully guided; faster atoms strike the tube wall and are lost from the beam.

  18. Optical molasses, laser traps, and ultracold atoms

    International Nuclear Information System (INIS)

    There is dramatic progress in the demonstration of the mechanical effects of light on atoms. The laser cooling and stopping of atoms in an atomic beam were followed by the 3-D cooling and confinement of atoms with laser light. The authors survey the recent major experimental advances and try to point out some interesting physics that can be done in this newly accessible domain of gaseous atoms at low temperatures and possibly high densities

  19. A slow gravity compensated atom laser

    DEFF Research Database (Denmark)

    Kleine Büning, G.; Will, J.; Ertmer, W.;

    2010-01-01

    We report on a slow guided atom laser beam outcoupled from a Bose–Einstein condensate of 87Rb atoms in a hybrid trap. The acceleration of the atom laser beam can be controlled by compensating the gravitational acceleration and we reach residual accelerations as low as 0.0027 g. The outcoupling me...

  20. Method And Apparatus For Atomizing And Vaporizing Liquid

    KAUST Repository

    Lal, Amit

    2014-09-18

    A method and apparatus for atomizing and vaporizing liquid is described. An apparatus having an ejector configured to eject one or more droplets of liquid may be inserted into a reservoir containing liquid. The ejector may have a vibrating device that vibrates the ejector and causes liquid to move from the reservoir up through the ejector and out through an orifice located on the top of the ejector. The one or more droplets of liquid ejected from the ejector may be heated and vaporized into the air.

  1. Towards laser-manipulated deposition for atom-scale technologies

    International Nuclear Information System (INIS)

    We have developed an apparatus for nanostructure fabrication based on direct deposition of laser-manipulated cesium vapors onto pyrolitic graphite. Key features of our apparatus are production and manipulation of a longitudinally cooled atom beam, which allows for straightforward operation in the moderate to low flux density conditions. Both unstructured and structured low surface coverage depositions have been carried out and samples carefully analyzed at the atom scale by in situ tunneling microscopy. Results represent a step forward to the realization of a novel technology for space-controlled deposition of few, eventually single, atoms.

  2. Diffusion of Rb atoms in paraffin - coated resonant vapor cells

    CERN Document Server

    Atutov, S N; Plekhanov, A I; Sorokin, V A; Yakovlev, A V

    2016-01-01

    We present the results of a study of the diffusion of Rb atoms in paraffin - coated resonant vapor cells. We have modeled the Rb diffusion both in the cell and in the coating, assuming that the main loss of Rb atoms is due to the physical absorption of the atoms by the glass substrate. It is demonstrated that the equilibrium atomic density in the cell is a monotonic function of the thickness of the paraffin coating: the density increases with an increase in the thickness of the coating. The diffusion coefficient for rubidium in paraffin thin films has been determined to be equal to 4,7*10^-7 cm^2/s. The results of the experiment might be useful for a better understanding of the details involved in the processes of the interaction of alkali atoms with a paraffin coating.

  3. An ultra-bright atom laser

    International Nuclear Information System (INIS)

    We present a novel, ultra-bright atom laser and an ultra-cold thermal atom beam. Using rf-radiation we strongly couple the magnetic hyperfine levels of 87Rb atoms in a trapped Bose–Einstein condensate. The resulting time-dependent adiabatic potential forms a trap, which at low rf-frequencies opens just below the condensate and thus allows an extremely bright well-collimated atom laser beam to emerge. As opposed to traditional atom lasers based on weak coupling of the magnetic hyperfine levels, this technique allows us to outcouple atoms at an arbitrarily large rate. We achieve a flux of 4×107 atom s-1, a seven fold increase compared to the brightest atom lasers to date. Furthermore, we demonstrate by two orders of magnitude the coldest thermal atom beam (200 nK). (paper)

  4. Experimental and theoretical studies of metal vapor atoms

    International Nuclear Information System (INIS)

    Employing electron spectrometry in conjunction with tuneable synchrotron radiation, we will present a detailed examination of the photoionization dynamics of selected metal vapor atoms. In particular, this paper will focus on the relative partial cross sections of the atomic Li K-shell main and satellite (ionization with excitation) photoelectron lines in the region of the strong 1snln'l' autoionizing transitions, the atomic Sc 3d, 4s main and satellite photoelectron lines in the region of the 3p→3d giant resonance, and also the atomic Fe 3d, 4s main and satellite photoelectron lines in the same resonance region. Our experimental data for Sc and Fe will be compared to our state-of-the-art calculations based on the superposition of configuration method developed by Cowan (The Theory of Atomic Structure and Spectra. University of California Berkeley Press, Berkeley and Los Angeles, 1981). Our partial cross section measurements for Li and Sc will be complemented with measurements of the angular distribution parameter, β. In addition, our Li data will also be compared with recent R-matrix calculations (Phys. Rev. 57 (1998) 1045). In the case of Fe, we will also address the term dependent behavior of the partial cross sections on resonance. These results will highlight what can be achieved with today's technology and point the way towards future endeavors in the study of the photoionization dynamics of open-shell metal vapor atoms

  5. Laser cooling and trapping of atoms

    International Nuclear Information System (INIS)

    The basic ideas of laser cooling and atom trapping will be discussed. These techniques have applications in spectroscopy, metrology, nuclear physics, biophysics, geophysics, and polymer science. (author)

  6. Laser manipulation of atoms and nanofabrication

    NARCIS (Netherlands)

    Jurdík, Erich

    2001-01-01

    Fundamental interaction processes between atoms and photons are exploited to control external degrees of freedom of the atoms. Laser light, when properly tuned near an atomic resonance, exerts such forces that the atoms are repelled from or attracted to the regions with low light intensities. We use

  7. Computer simulated rate processes in copper vapor lasers

    Science.gov (United States)

    Harstad, K. C.

    1980-01-01

    A computer model for metal vapor lasers has been developed which places emphasis on the change of excited state populations of the lasant through inelastic collisions and radiative interaction. Also included are an energy equation for the pumping electrons and rate equations for laser photon densities. Presented are results of calculations for copper vapor with a neon buffer over a range of conditions. General agreement with experiments was obtained.

  8. Atomic vapor laser isotope separation in France

    International Nuclear Information System (INIS)

    The main effort in the field of Isotopic Separation Research and Development in France is devoted since 1985 to the 'SILVA' process. A structured organization has been set up, including the following elements: Specific Research and Development for all the functions and components of the process: this work is supported by numerous benches located in Saclay and Pierrelatte. Each bench is mainly devoted to one process function; regarding process and operating performances are optimized. Integrated Experiences in a Pilot facility. Qualified components are integrated in a pilot facility located in Saclay, the capacity of which is steadily increased. At each stage, complete separative experiments demonstrate the improvements attained. Focused Basic Research for each field, often linked with various and relatively original phenomenas. Models have been built up, supported by specific experiments and values attained for intrinsical parameters. An aggregated process performance computing code integrates all the models, possibly under simplified form. Technical, operating and economical data are gradually added. A general assessment will take place in the middle of the nineties with several technical demonstrations and a complete evaluation of the French AVLIS process

  9. Trace direction of plutonium by three-step photoionization with a laser system pumped by a copper vapor laser

    International Nuclear Information System (INIS)

    Laser photoionization has been used to detect trace amounts of plutonium. A high sensitivity and selectivity has been achieved by applying three-step excitation and ionization of the plutonium atoms with high pulse-repetition rates and additional mass determination by time-of-flight measurements. A laser system was developed which consists of a copper vapor laser pumping three dye lasers simultaneously. Samples containing between 1010 and 1012 atoms of 239Pu on Re filaments were measured yielding strong resonance signals with maximum ion count rates of several kHz at a vanishingly low background. A detection efficiency of 10-7 was determined allowing the detection of about 108 plutonium atoms in a sample. (orig.)

  10. Heterodyne phase shift diagnostic for measuring atomic vapor density

    International Nuclear Information System (INIS)

    We describe a technique for atomic density measurements. We generate and recombine frequency shifted laser beams producing beat signals on reference and signal detectors. Opacity in the signal detector leg is proportional to the phase difference between detector signals. 4 refs., 2 figs

  11. Coupling a thermal atomic vapor to an integrated ring resonator

    CERN Document Server

    Ritter, Ralf; Pernice, Wolfram; Kübler, Harald; Pfau, Tilman; Löw, Robert

    2016-01-01

    Strongly interacting atom-cavity systems within a network with many nodes constitute a possible realization for a quantum internet which allows for quantum communication and computation on the same platform. To implement such large-scale quantum networks, nanophotonic resonators are promising candidates because they can be scalably fabricated and interconnected with waveguides and optical fibers. By integrating arrays of ring resonators into a vapor cell we show that thermal rubidium atoms above room temperature can be coupled to photonic cavities as building blocks for chip-scale hybrid circuits. Although strong coupling is not yet achieved in this first realization, our approach provides a key step towards miniaturization and scalability of atom-cavity systems.

  12. Isotropic Negatively-Refracting Atomic-Vapor Medium

    Science.gov (United States)

    Shen, Jian Qi

    A new scenario to realize negative refraction with a photonic-resonant vapor material that can exhibit both electric and magnetic responses via multilevel quantum coherence is suggested. Compared with the previous method of artificial composite metamaterial, where the mechanism was considered by means of classical electromagnetic theory and the materials produced have anisotropic millimetre-scale composite structures, the present scheme suggested within the framework of quantum optics can be used to design and fabricate isotropic negatively-refracting materials with atomic-scale microscopic structure units. Such an advantage may lead to a potentially important application in the techniques of superlens and perfect imaging.

  13. Modeling atomization processes in high-pressure vaporizing sprays

    Science.gov (United States)

    Reitz, Rolf D.

    The theoretical basis and numerical implementation of KIVA, a multidimensional computer code for the simulation of atomization and vaporization processes in the injection of a liquid through a round hole into a compressed gas, are described. KIVA is based on the blob-injection model of Reitz and Diwakar (1987), taking into account the effects of liquid inertia, surface tension, and the aerodynamic forces on the jet, as well as drop collision and coalescence and the effect of drops on turbulence in the gas. The predictions of KIVA for different injection regimes are compared with published experimental data in extensive graphs, and good agreement is demonstrated.

  14. Single Molecule DNA Detection with an Atomic Vapor Notch Filter

    CERN Document Server

    Uhland, Denis; Widmann, Matthias; Lee, Sang-Yun; Wrachtrup, Jörg; Gerhardt, Ilja

    2015-01-01

    The detection of single molecules has facilitated many advances in life- and material-sciences. Commonly, it founds on the fluorescence detection of single molecules, which are for example attached to the structures under study. For fluorescence microscopy and sensing the crucial parameters are the collection and detection efficiency, such that photons can be discriminated with low background from a labeled sample. Here we show a scheme for filtering the excitation light in the optical detection of single stranded labeled DNA molecules. We use the narrow-band filtering properties of a hot atomic vapor to filter the excitation light from the emitted fluorescence of a single emitter. The choice of atomic sodium allows for the use of fluorescent dyes, which are common in life-science. This scheme enables efficient photon detection, and a statistical analysis proves an enhancement of the optical signal of more than 15% in a confocal and in a wide-field configuration.

  15. An atom laser based on Raman transitions

    CERN Document Server

    Moy, G M; Savage, C M

    1996-01-01

    In this paper we present an atom laser scheme using a Raman transition for the output coupling of atoms. A beam of thermal atoms (bosons) in a metastable atomic state |1> are pumped into a multimode atomic cavity. This cavity is coupled through spontaneous emission to a single mode of another cavity for the ground atomic state, |2>. Above a certain threshold pumping rate a large number of atoms, N2, builds up in this single quantum state and transitions to the ground state of the cavity become enhanced by a factor (N2+1). Atoms in this state are then coupled to the outside of the cavity with a Raman transition. This changes the internal state of the atom and imparts a momentum kick, allowing the atoms to leave the system.

  16. A resonance ionization imaging detector based on cesium atomic vapor

    International Nuclear Information System (INIS)

    A novel Cs resonance ionization imaging detector (RIID) has been developed and evaluated. The detector is capable of two-dimensional imaging with high spectral resolution, which is determined by the Doppler broadened atomic linewidth of Cs at given temperature. Ionization schemes of Cs have been investigated using dye and color center tunable lasers pumped by an excimer laser and by a Nd:YAG laser. It has been experimentally shown that the most efficient ionization scheme for Cs RIID should include a three-step excitation/ionization ladder, for example, with transitions at λ1=852.11 (852.113) nm, λ2=917.22 (917.2197) nm, and λ3=1064 nm. The imaging capabilities of the detector have been evaluated using a simpler two-step ionization scheme with wavelengths λ1=852.11 nm and λ2=508 nm

  17. A resonance ionization imaging detector based on cesium atomic vapor

    Science.gov (United States)

    Temirov, J. P.; Chigarev, N. V.; Matveev, O. I.; Omenetto, N.; Smith, B. W.; Winefordner, J. D.

    2004-05-01

    A novel Cs resonance ionization imaging detector (RIID) has been developed and evaluated. The detector is capable of two-dimensional imaging with high spectral resolution, which is determined by the Doppler broadened atomic linewidth of Cs at given temperature. Ionization schemes of Cs have been investigated using dye and color center tunable lasers pumped by an excimer laser and by a Nd:YAG laser. It has been experimentally shown that the most efficient ionization scheme for Cs RIID should include a three-step excitation/ionization ladder, for example, with transitions at λ1=852.11 (852.113) nm, λ2=917.22 (917.2197) nm, and λ3=1064 nm. The imaging capabilities of the detector have been evaluated using a simpler two-step ionization scheme with wavelengths λ1=852.11 nm and λ2=508 nm.

  18. Laser plasma channel formation in barium vapor based on superelastic heating of electrons

    International Nuclear Information System (INIS)

    Computational study of plasma channel formation kinetics in optically dense barium vapor irradiated by pulsed laser light tuned to the Ba I resonance transition at λ = 553.5 nm has been performed. Seed electrons are produced due to the mechanism of atoms associative ionization, which then gain energy in superelastic collisions and initiate the avalanche ionization of atoms by electron impact. We have studied the influence of radiative transfer effects in cylindrically symmetric gas volume on the excitation kinetics of multilevel barium atoms, dynamics of absorption of laser radiation, and the plasma channel expansion in the form of a halo in condition of competition between the ionizing and quenching electron collisions with excited atoms. (paper)

  19. Effect of surrounding gases and water vapor on the induced electric current associated with a laser-induced plasma

    Science.gov (United States)

    Matsuta, Hideyuki

    2016-04-01

    The effect of surrounding gases and water vapor on the laser-induced electric current was investigated. Laser-induced plasma was generated on an aluminum alloy target. The laser-induced plasma was optically examined to estimate the excitation temperature and electron density in room air. There was a linear relationship between the maximum amplitude of the laser-induced current and the electron density. As the electron mean free path of the surrounding gas increased, the observed amplitude of the current increased. The amplitude of the induced current signal in dry air became maximum upon mixing with the optimum amount of water vapor. This enhancement of the induced current signal might be due to the large relative permittivity of water vapor. The laser-induced plasma as a whole seems to be a low-temperature plasma consisting of electrons, a large amount of cold surrounding gas, injected hot atoms, hot ions, and hot particles.

  20. Theoretical tools for atom laser beam propagation

    OpenAIRE

    Riou, J. -F.; Coq, Y. Le; Impens, F; Guerin, W.; Bordé, C. J.; Aspect, A; Bouyer, P.

    2008-01-01

    We present a theoretical model for the propagation of non self-interacting atom laser beams. We start from a general propagation integral equation, and we use the same approximations as in photon optics to derive tools to calculate the atom laser beam propagation. We discuss the approximations that allow to reduce the general equation whether to a Fresnel-Kirchhoff integral calculated by using the stationary phase method, or to the eikonal. Within the paraxial approximation, we also introduce...

  1. Observation of nonlinear laser spectra of cold atoms in diffuse light

    CERN Document Server

    Zhang, Wen-zhuo; Liu, Liang; Wang, Yu-zhu

    2009-01-01

    The recoil-induced resonances (RIR) and electromagnetic-induced absorption (EIA) are observed in an experiment of diffuse cooling of $^{87}$Rb atomic vapor in an integrating sphere. We measured the nonlinear spectra varying with detuning of the diffuse laser light, and study their mechanism in the diffuse-light pumped and laser-beam probed configuration. Their differences from nonlinear spectra of cold atoms in one-dimensional optical molasses and magneto-optical trap (MOT) are also discussed.

  2. Enthalpy model for heating, melting, and vaporization in laser ablation

    OpenAIRE

    Vasilios Alexiades; David Autrique

    2010-01-01

    Laser ablation is used in a growing number of applications in various areas including medicine, archaeology, chemistry, environmental and materials sciences. In this work the heat transfer and phase change phenomena during nanosecond laser ablation of a copper (Cu) target in a helium (He) background gas at atmospheric pressure are presented. An enthalpy model is outlined, which accounts for heating, melting, and vaporization of the target. As far as we know, this is the first model th...

  3. Sub-picotesla Scalar Atomic Magnetometer with a Microfabricated Vapor Cell

    Science.gov (United States)

    Zhang, Rui; Mhaskar, Rahul

    2016-05-01

    We explore the sensitivity limits of scalar atomic magnetometry with a micro-fabricated Cs vapor cell. The millimeter-scale cell is fabricated using silicon Micro-Electro-Mechanical Systems (MEMS) technology. The atomic spin procession is driven by an amplitude-modulated circularly polarized pump laser resonant with the D1 transition in Cs atoms. The precession is detected by an off-resonant linearly polarized probe laser using a balanced polarimeter setup. The probe light is spatially split into two beams to perform a gradiometer measurement. In a magnetic field of magnitude within the range of the earth magnetic field, we measure a sensitivity of less than 150 fT/ √Hz in the gradiometer mode, which shows that the magnetometer by itself can achieve sub-100 fT/ √Hz sensitivitiy. In addition to its high sensitivity, the magnetometer has a bandwidth of nearly 1 kHz due to the broad magnetic resonance inside the small cell. Our experiment suggests the feasibility of a portable, low-power and high-performance magnetometer, which can be operated in the earth's magnetic field. Such a device will greatly expand the range of applications for atomic magnetometers, such as the detection of nuclear magnetic resonance in an unshielded environment.

  4. Diode Pumped Alkali Vapor Lasers - A New Pathway to High Beam Quality at High Average Power

    Energy Technology Data Exchange (ETDEWEB)

    Page, R H; Boley, C D; Rubenchik, A M; Beach, R J

    2005-05-06

    Resonance-transition alkali-vapor lasers have only recently been demonstrated [1] but are already attracting considerable attention. Alkali-atom-vapor gain media are among the simplest possible systems known, so there is much laboratory data upon which to base performance predictions. Therefore, accurate modeling is possible, as shown by the zero- free-parameter fits [2] to experimental data on alkali-vapor lasers pumped with Ti:sapphire lasers. The practical advantages of two of the alkali systems--Rb and Cs--are enormous, since they are amenable to diode-pumping [3,4]. Even without circulating the gas mixture, these lasers can have adequate cooling built-in owing to the presence of He in their vapor cells. The high predicted (up to 70%) optical-to-optical efficiency of the alkali laser, the superb (potentially 70% or better) wall-plug efficiency of the diode pumps, and the ability to exhaust heat at high temperature (100 C) combine to give a power-scalable architecture that is lightweight. A recent design exercise [5] at LLNL estimated that the system ''weight-to-power ratio'' figure of merit could be on the order of 7 kg/kW, an unprecedented value for a laser of the 100 kW class. Beam quality is expected to be excellent, owing to the small dn/dT value of the gain medium. There is obviously a long way to go, to get from a small laser pumped with a Ti:sapphire or injection-seeded diode system (of near-perfect beam quality, and narrow linewidth) [1, 4] to a large system pumped with broadband, multimode diode- laser arrays. We have a vision for this technology-development program, and have already built diode-array-pumped Rb lasers at the 1 Watt level. A setup for demonstrating Diode-array-Pumped Alkali vapor Lasers (DPALs) is shown in Figure 1. In general, use of a highly-multimode, broadband pump source renders diode-array-based experiments much more difficult than the previous ones done with Ti:sapphire pumping. High-NA optics, short focal

  5. Experimental study of vapor-cell magneto-optical traps for efficient trapping of radioactive atoms

    International Nuclear Information System (INIS)

    We have studied magneto-optical traps (MOTs) for efficient on-line trapping of radioactive atoms. After discussing a model of the trapping process in a vapor cell and its efficiency, we present the results of detailed experimental studies on Rb MOTs. Three spherical cells of different sizes were used. These cells can be easily replaced, while keeping the rest of the apparatus unchanged: atomic sources, vacuum conditions, magnetic field gradients, sizes and power of the laser beams, detection system. By direct comparison, we find that the trapping efficiency only weakly depends on the MOT cell size. It is also found that the trapping efficiency of the MOT with the smallest cell, whose diameter is equal to the diameter of the trapping beams, is about 40% smaller than the efficiency of larger cells. Furthermore, we also demonstrate the importance of two factors: a long coated tube at the entrance of the MOT cell, used instead of a diaphragm; and the passivation with an alkali vapor of the coating on the cell walls, in order to minimize the losses of trappable atoms. These results guided us in the construction of an efficient large-diameter cell, which has been successfully employed for on-line trapping of Fr isotopes at INFN's national laboratories in Legnaro, Italy. (authors)

  6. Modeling a semiconductor laser with an intracavity atomic absorber

    International Nuclear Information System (INIS)

    The dynamics of a semiconductor laser with an intracavity atomic absorber is studied numerically. The study is motivated by the experiments of Barbosa et al. [Opt. Lett. 32, 1869 (2007)], using a semiconductor junction as an active medium, with its output face being antireflection coated, and a cell containing cesium vapor placed in a cavity that was closed by a diffraction grating (DG). The DG allowed scanning the lasing frequency across the D2 line in the Cs spectrum, and different regimes such as frequency bistability or dynamic instability were observed depending on the operating conditions. Here we propose a rate-equation model that takes into account the dispersive losses and the dispersive refractive index change in the laser cavity caused by the presence of the Cs vapor cell. These effects are described through a modification of the complex susceptibility. The numerical results are found to be in qualitative good agreement with some of the observations; however, some discrepancies are also noticed, which can be attributed to multi-longitudinal-mode emission in the experiments. The simulations clearly show the relevant role of the Lamb dips and crossover resonances, which arise on top of the Doppler-broadened D2 line in the Cs spectrum, and are due to the forward and backward intracavity fields interacting resonantly with the Cs atoms. When the laser frequency is locked in a dip, a reduction in the frequency noise and of the intensity noise is demonstrated.

  7. Laser stabilization to an atomic transition using an optically generated dispersive lineshape

    CERN Document Server

    Queiroga, Fabiano; Mestre, Valdeci; Vidal, Itamar; de Silans, Thierry Passerat; Oriá, Marcos; Chevrollier, Martine

    2012-01-01

    We report on a simple and robust technique to generate a dispersive signal which serves as an error signal to electronically stabilize a monomode cw laser emitting around an atomic resonance. We explore nonlinear effects in the laser beam propagation through a resonant vapor by way of spatial filtering. The performance of this technique is validated by locking semiconductor lasers to the cesium and rubidiumD2 line and observing long-term reduction of the emission frequency drifts, making the laser well adapted for many atomic physics applications.

  8. Bose-Einstein condensation in a vapor of sodium atoms in an electric field

    Science.gov (United States)

    You, Pei-Lin

    2016-06-01

    Bose-Einstein condensation (BEC) at normal temperature (T=343K) has been observed because an electric field was first applied. There are two ways to achieve phase transition: lower the temperature of Bose gas or increase its density. This article provides more appropriate method: increase the voltage. In theory, 3s and 3p states of sodium are not degenerate, but Na may be polar atom doesnot conflict with quantum mechanics because it is hydrogen-like atom. Our innovation lies in we applied an electric field used for the orientation polarization. Na vapor was filled in a cylindrical capacitor. In order to determine the polarity of sodium, we measured the capacitance at different temperatures. If Na is non-polar atom, its capacitance should be independent of temperature because the nucleus of atom is located at the center of the electron cloud. But our experiment shows that its capacitance is related to temperature, so Na is polar atom. In order to achieve Na vapor phase transition, we measured the capacitance at different voltages. From the entropy of Na vapor S=0, the critical voltage Vc=68volts. When V0; when V>Vc, the atoms become aligned with the field Svapor entered quasi-vacuum state. We create a BEC with 2.506×1017 atoms, condensate fraction reached 98.9%. This is BEC in momentum space. Our experiment shows that if a Bose gas enters quasi-vacuum state, this also means that it underwent phase transition and generates BEC. Therefore, quasi-vacuum state of alkali gas is essentially large-scale BEC. This is an unexpected discovery. BEC and vacuum theory are two unrelated research areas, but now they are closely linked together. The maximum induced dipole moment dind≤7.8×10-15 e cm can be neglected. Ultra-low temperature is in order to make Bose gas phase transition, we achieve the phase transition by the critical voltage, so the ultra-low temperature is not necessary. According to the standard proposed by Ketterle, although we didn't use laser cooling atoms

  9. Nd:Glass-Raman laser for water vapor dial

    Science.gov (United States)

    Kagann, R. H.; Petheram, J. C.; Rosenberg, A.

    1986-01-01

    A tunable solid-state Raman shifted laser which was used in a water vapor Differential Absorption Lidar (DIAL) system at 9400 A is described. The DIAL transmitter is based on a tunable glass laser operating at 1.06 microns, a hydrogen Raman cell to shift the radiation to 1.88 microns, and a frequency doubling crystal. The results of measurements which characterize the output of the laser with respect to optimization of optical configuration and of Raman parameters were reported. The DIAL system was also described and preliminary atmospheric returns shown.

  10. Growth of Carbon Nanostructure Materials Using Laser Vaporization

    Science.gov (United States)

    Zhu, Shen; Su, Ching-Hua; Lehozeky, S.

    2000-01-01

    Since the potential applications of carbon nanotubes (CNT) was discovered in many fields, such as non-structure electronics, lightweight composite structure, and drug delivery, CNT has been grown by many techniques in which high yield single wall CNT has been produced by physical processes including arc vaporization and laser vaporization. In this presentation, the growth mechanism of the carbon nanostructure materials by laser vaporization is to be discussed. Carbon nanoparticles and nanotubes have been synthesized using pulsed laser vaporization on Si substrates in various temperatures and pressures. Two kinds of targets were used to grow the nanostructure materials. One was a pure graphite target and the other one contained Ni and Co catalysts. The growth temperatures were 600-1000 C and the pressures varied from several torr to 500 torr. Carbon nanoparticles were observed when a graphite target was used, although catalysts were deposited on substrates before growing carbon films. When the target contains catalysts, carbon nanotubes (CNT) are obtained. The CNT were characterized by scanning electron microscopy, x-ray diffraction, optical absorption and transmission, and Raman spectroscopy. The temperature-and pressure-dependencies of carbon nanotubes' growth rate and size were investigated.

  11. Theory of optical near-resonant cone emission in atomic vapor

    International Nuclear Information System (INIS)

    A time-dependent theory for conical emission during near-resonant propagation of laser light in an atomic vapor, which includes full propagation for the laser and frequency sidebands in a nonlinear two-level medium is presented. The density-matrix equations for the dipole moment and population are solved in the dressed atomic frame. The polarization source terms are accurate to order γ/R, where γ is a damping constant and R is the generalized Rabi frequency. Analytical plane-wave solutions and numerical, cylindrically symmetric propagation simulations including diffraction are presented. It is shown that the calculations with cylindrically symmetric fields and atomic excitation profiles are incapable of accounting for the high levels of optical gain that are responsible for the intense conical emission observed in experiments. This result is at first surprising, since the model accounts rigorously for all of the physical phenomena that have been previously proposed as being responsible for generating large gains, and the calculation matches the symmetry of the observations. The lack of large calculated gain seems to imply the existence of higher-order (m>0) radial modes in the field for the experimental conditions that give rise to cone emission. In the simulations, however, the cylindrically symmetric fields do produce weak red-detuned cones with angular-frequency distributions similar to those seen in experiments

  12. Dual-axis vapor cell for simultaneous laser frequency stabilization on disparate optical transitions

    International Nuclear Information System (INIS)

    We have developed a dual-axis ytterbium (Yb) vapor cell and used it to simultaneously address the two laser cooling transitions in Yb at wavelengths 399 nm and 556 nm, featuring the disparate linewidths of 2π × 29 MHz and 2π × 182 KHz, respectively. By utilizing different optical paths for the two wavelengths, we simultaneously obtain comparable optical densities suitable for saturated absorption spectroscopy for both the transitions and keep both the lasers frequency stabilized over several hours. We demonstrate that by appropriate control of the cell temperature profile, two atomic transitions differing in relative strength across a large range of over three orders of magnitude can be simultaneously addressed, making the device adaptable to a variety of spectroscopic needs. We also show that our observations can be understood with a simple theoretical model of the Yb vapor

  13. Dual-axis vapor cell for simultaneous laser frequency stabilization on disparate optical transitions

    Science.gov (United States)

    Jayakumar, Anupriya; Plotkin-Swing, Benjamin; Jamison, Alan O.; Gupta, Subhadeep

    2015-07-01

    We have developed a dual-axis ytterbium (Yb) vapor cell and used it to simultaneously address the two laser cooling transitions in Yb at wavelengths 399 nm and 556 nm, featuring the disparate linewidths of 2π × 29 MHz and 2π × 182 KHz, respectively. By utilizing different optical paths for the two wavelengths, we simultaneously obtain comparable optical densities suitable for saturated absorption spectroscopy for both the transitions and keep both the lasers frequency stabilized over several hours. We demonstrate that by appropriate control of the cell temperature profile, two atomic transitions differing in relative strength across a large range of over three orders of magnitude can be simultaneously addressed, making the device adaptable to a variety of spectroscopic needs. We also show that our observations can be understood with a simple theoretical model of the Yb vapor.

  14. Conservation laws and laser cooling of atoms

    Science.gov (United States)

    Giuliani, Giuseppe

    2015-11-01

    The straightforward application of energy and linear momentum conservation to the absorption/emission of photons by atoms allows us to establish the essential features of laser cooling of two level atoms at low laser intensities. The lowest attainable average kinetic energy of the atoms depends on the ratio {{Γ }}/{E}{{R}} between the natural linewidth and the recoil energy and tends to ER as {{Γ }}/{E}{{R}} tends to zero (in one dimension). This treatment, like the quantum mechanical ones, is valid for any value of the ratio {{Γ }}/{E}{{R}} and contains the semiclassical theory of laser cooling as the limiting case in which {E}{{R}}\\ll {{Γ }}.

  15. Laser trapping of 21Na atoms

    International Nuclear Information System (INIS)

    This thesis describes an experiment in which about four thousand radioactive 21Na (tl/2 = 22 sec) atoms were trapped in a magneto-optical trap with laser beams. Trapped 21Na atoms can be used as a beta source in a precision measurement of the beta-asymmetry parameter of the decay of 21Na → 21Ne + Β+ + ve, which is a promising way to search for an anomalous right-handed current coupling in charged weak interactions. Although the number o trapped atoms that we have achieved is still about two orders of magnitude lower than what is needed to conduct a measurement of the beta-asymmetry parameter at 1% of precision level, the result of this experiment proved the feasibility of trapping short-lived radioactive atoms. In this experiment, 21Na atoms were produced by bombarding 24Mg with protons of 25 MeV at the 88 in. Cyclotron of Lawrence Berkeley Laboratory. A few recently developed techniques of laser manipulation of neutral atoms were applied in this experiment. The 21Na atoms emerging from a heated oven were first transversely cooled. As a result, the on-axis atomic beam intensity was increased by a factor of 16. The atoms in the beam were then slowed down from thermal speed by applying Zeeman-tuned slowing technique, and subsequently loaded into a magneto-optical trap at the end of the slowing path. The last two chapters of this thesis present two studies on the magneto-optical trap of sodium atoms. In particular, the mechanisms of magneto-optical traps at various laser frequencies and the collisional loss mechanisms of these traps were examined

  16. Laser beam propagation effects in atomic laser isotope separation

    International Nuclear Information System (INIS)

    The propagation of two different-color laser pulses in the resonant three-level medium is studied. The three-level Bloch-Maxwell equations are solved numerically to analyze the change of the pulse shapes and the time-varying atomic populations. The pulse delay and the pulse shape break-up are observed especially for the first excitation laser pulse. Complete separation of the two laser pulses occur from a certain critical distance. It is shown that the rapid decrease of the ionization efficiency is caused by the separation of the two laser pulses. (author)

  17. Towards a random laser with cold atoms

    CERN Document Server

    Guerin, William; Michaud, Franck; Brivio, Davide; Froufe-Pérez, Luis S; Carminati, Rémi; Eremeev, Vitalie; Goetschy, Arthur; Skipetrov, Sergey S; Kaiser, Robin

    2009-01-01

    Atoms can scatter light and they can also amplify it by stimulated emission. From this simple starting point, we examine the possibility of realizing a random laser in a cloud of laser-cooled atoms. The answer is not obvious as both processes (elastic scattering and stimulated emission) seem to exclude one another: pumping atoms to make them behave as amplifier reduces drastically their scattering cross-section. However, we show that even the simplest atom model allows the efficient combination of gain and scattering. Moreover, supplementary degrees of freedom that atoms offer allow the use of several gain mechanisms, depending on the pumping scheme. We thus first study these different gain mechanisms and show experimentally that they can induce (standard) lasing. We then present how the constraint of combining scattering and gain can be quantified, which leads to an evaluation of the random laser threshold. The results are promising and we draw some prospects for a practical realization of a random laser wit...

  18. Phase dynamics in a binary-collisions atom laser scheme

    OpenAIRE

    Zobay, O.; Meystre, P.

    1997-01-01

    Various aspects of the phase dynamics of an atom laser scheme based on binary collisions are investigated. Analytical estimates of the influence of elastic atom-atom collisions on the laser linewidth are given, and linewidths achievable in a recently proposed atom laser scheme [Phys. Rev. A 56, 2989 (1997)] are evaluated explicitly. The extent to which a relative phase can be established between two interfering atom lasers, as well as the properties of that phase, are also investigated.

  19. Magnetically tuned, robust and efficient filtering system for spatially multimode quantum memory in warm atomic vapors

    CERN Document Server

    Dąbrowski, Michał; Wasilewski, Wojciech

    2015-01-01

    Warm atomic vapor quantum memories are simple and robust, yet suffer from a number of parasitic processes which produce excess noise. For operating in a single-photon regime precise filtering of the output light is essential. Here we report a combination of magnetically tuned absorption and Faraday filters, both light-direction-insensitive, which stop the driving lasers and attenuate spurious fluorescence and four-wave mixing while transmitting narrowband Stokes and anti-Stokes photons generated in write-in and readout processes. We characterize both filters with respect to adjustable working parameters. We demonstrate a significant increase in the signal to noise ratio upon applying the filters seen qualitatively in measurements of correlation between the Raman-scattered photons.

  20. Narrow linewidth single laser source system for onboard atom interferometry

    OpenAIRE

    Theron, Fabien; Carraz, Olivier; Renon, Geoffrey; Bidel, Yannick; Zahzam, Nassim; Cadoret, Malo; Bresson, Alexandre

    2014-01-01

    A compact and robust laser system for atom interferometry based on a frequency-doubled telecom laser is presented. Thanks to an original stabilization architecture on a saturated absorption setup, we obtain a frequency-agile laser system allowing fast tuning of the laser frequency over 1 GHz in few ms using a single laser source. The different laser frequencies used for atom interferometry are generated by changing dynamically the frequency of the laser and by creating sidebands using a phase...

  1. Laser Spectroscopy of Antiprotonic Helium Atoms

    CERN Multimedia

    2002-01-01

    %PS205 %title\\\\ \\\\Following the discovery of metastable antiprotonic helium atoms ($\\overline{p}He^{+} $) at KEK in 1991, systematic studies of their properties were made at LEAR from 1991 to 1996. In the first two years the lifetime of $\\overline{p}He^{+}$ in liquid and gaseous helium at various temperatures and pressures was measured and the effect of foreign gases on the lifetime of these atoms was investigated. Effects were also discovered which gave the antiproton a 14\\% longer lifetime in $^4$He than in $^3$He, and resulted in important differences in the shape of the annihilation time spectra in the two isotopes.\\\\ \\\\Since 1993 laser spectroscopy of the metastable $\\overline{p}He^{+}$ atoms became the main focus of PS205. Transitions were stimulated between metastable and non-metastable states of the $\\overline{p}He^{+}$ atom by firing a pulsed dye laser beam into the helium target every time an identified metastable atom was present (Figure 1). If the laser frequency matched the transition energy, the...

  2. Alloying element vaporization during laser spot welding of stainless steel

    International Nuclear Information System (INIS)

    Alloying element loss from the weld pool during laser spot welding of stainless steel was investigated experimentally and theoretically. The experimental work involved determination of work-piece weight loss and metal vapour composition for various welding conditions. The transient temperature and velocity fields in the weld pool were numerically simulated. The vaporization rates of the alloying elements were modelled using the computed temperature profiles. The fusion zone geometry could be predicted from the transient heat transfer and fluid flow model for various welding conditions. The laser power and the pulse duration were the most important variables in determining the transient temperature profiles. The velocity of the liquid metal in the weld pool increased with time during heating and convection played an increasingly important role in the heat transfer. The peak temperature and velocity increased significantly with laser power density and pulse duration. At very high power densities, the computed temperatures were higher than the boiling point of 304 stainless steel. As a result, evaporation of alloying elements was caused by both the total pressure and the concentration gradients. The calculations showed that the vaporization occurred mainly from a small region under the laser beam where the temperatures were very high. The computed vapour loss was found to be lower than the measured mass loss because of the ejection of tiny metal droplets owing to the recoil force exerted by the metal vapours. The ejection of metal droplets has been predicted by computations and verified by experiments

  3. Carbon-atom wires produced by nanosecond pulsed laser deposition in a background gas

    OpenAIRE

    Casari, C. S.; Giannuzzi, C. S.; V. Russo

    2016-01-01

    Wires of sp-hybridized carbon atoms are attracting interest for both fundamental aspects of carbon science and for their appealing functional properties. The synthesis by physical vapor deposition has been reported to provide sp-rich carbon films but still needs to be further developed and understood in detail. Here the synthesis of carbon-atom wires (CAWs) has been achieved by nanosecond pulsed laser deposition (PLD) expoliting the strong out-of-equilibrium conditions occurring when the abla...

  4. Separating uranium by laser: the atomic process

    International Nuclear Information System (INIS)

    Among the countries around the world that utilizes nuclear energy, several ones are investing significantly in the development of laser techniques applied to isotope separation. In Brazil these studies are concentrated in one research institute, the IEAv (Institute for Advanced Studies), and aim at demonstrating the viability of this process using, as much as possible, resources available in the country. In this paper we briefly describe the laser methods for isotope separation, giving an overview of the present research and development status in this area. We also show some results obtained our laboratories. We focused this report on the atomic route for laser isotope separation, mainly in the areas of laser development and spectroscopy. (author)

  5. Continuous magnetic trapping of laser cooled atoms

    International Nuclear Information System (INIS)

    The authors present here initial results of the deceleration of a thermal atomic beam from -- 1000 to -- 100 m/s. The experiment was conducted in the 1.4-m long vertical superconducting solenoid which produced the slowing field. The fluorescence of the slowed atomic beam has been studied as a function of laser frequency. Figure 2 is a 12-GHz scan showing the fluorescence at a position 150 cm from the beginning of the solenoid. The wide peak corresponds to unslowed atoms with generally the initial velocity distribution. The second, narrower, peak corresponds to slowed atoms with a velocity of -- 150 m/s. Similar spectra have been obtained for various positions along the magnetic slower and trap. These data should allow better understanding of the cooling process and will be compared to computer models

  6. Self-organized subwavelength ripple by nanosecond laser induced chemical vapor deposition

    International Nuclear Information System (INIS)

    Polymeric hydrogenated amorphous carbon (α-C:H) thin films were prepared by laser induced chemical vapor deposited method using a KrF excimer laser (λ = 248 nm, Ofwhm = 25 ns) with different laser intensities. Field emission scanning electron microscopy and atomic force microscopy were used to investigate the surface morphology of the films. It was found that the surface morphologies were affected by the laser intensity significantly. Self-organized subwavelength fine ripples perpendicular to the laser beam polarization with periodicities of about 200 nm were observed and a reasonable explanation was proposed for the formation of the ripples. Raman spectroscopy and Fourier transform infrared spectroscopy were used to study the structure of the α-C:H films. The results suggested that there was oxygen in the films, which came from the ambient contamination and the incomposited impurities during and after deposition. The relationships between the composition and chemical bond types were discussed in detail. - Highlights: • Polymeric α-C:H thin films prepared by laser induced CVD with the laser wavelength of 248 nm • Fine ripples with periodicities of about 200 nm observed on the surface of the films • Composition and chemical bonds studied by Raman and Fourier transform infrared spectroscopy

  7. Semiclassical treatment of laser excitation of the hydrogen atom

    DEFF Research Database (Denmark)

    Billing, Gert D.; Henriksen, Niels Engholm; Leforestier, C.

    1992-01-01

    We present an alternative method for studying excitation of atoms in intense laser fields. In the present paper we focus upon the optical harmonic generation by hydrogen atoms.......We present an alternative method for studying excitation of atoms in intense laser fields. In the present paper we focus upon the optical harmonic generation by hydrogen atoms....

  8. Laser spectroscopy of multi-level doppler broadened atomic system

    International Nuclear Information System (INIS)

    Doppler broadened atomic vapor system can be easily prepared for spectroscopy study than an atomic beam system can be. Vapor cell and hollow cathode discharge lamps are widely used in the experiment. The possibility for observing the trapped state in a Doppler broadened Λ system was examined and confirmed by our early experiment where counter-propagating laser beams are used. For the measurement of the hyperfine structure constants of high-lying levels of heavy elements, we compared the co-propagating and counter-propagating beams in a Doppler broadened ladder systems. It was shown that the counter-propagating beams give a stronger and narrower signal than that from the co-propagating beams. Our treatment also considers the power broadening of the transition. For some photo-ionization experiments, it is necessary to pump two thermally populated levels simultaneously to the higher level and then to the auto-ionizing levels. A technique is proposed to avoid the trapped state and to increase the ionization efficiency.

  9. Electric and magnetic dipole allowed transitions of atoms for three-dimensionally isotropic left handedness in a mixed atomic vapor

    Science.gov (United States)

    Shen, Jian Qi

    2014-03-01

    Since previous negative-index atomic media based on quantum optical approaches are highly lossy, a proposal for realizing a three-dimensionally isotropic left-handed atomic vapor medium is suggested based on a mechanism of incoherent gain assisted atomic transitions. Two three-level atomic systems are utilized for producing simultaneously negative permittivity and negative permeability, respectively, in the same frequency band. We suggest that fine and hyperfine level transitions of atoms (e.g., a hyperfine level transition in a hydrogen atomic system and a fine level transition in an alkali-metal atomic system) would be applicable to realization of such a negatively refracting atomic vapor. The attractive features of the present scenario include: i) three-dimensionally isotropic negative indices; ii) incoherent gain wave amplification in the negative-index atomic vapor; iii) tunable negative indices depending upon external fields. Such a left-handed quantum optical medium can serve as a supporting substrate for lossy negative-index materials for loss compensation. It can also be used in designing new quantum optical and photonic devices (e.g., a subwavelength focusing system and a negative-index superlens for perfect imaging) because of its attractive properties of three-dimensional isotropy and high-gain wave amplification.

  10. Simple and Compact Nozzle Design for Laser Vaporization Sources

    CERN Document Server

    Kokish, M G; Odom, B C

    2015-01-01

    We have developed and implemented a compact transparent nozzle for use in laser vaporization sources. This nozzle eliminates the need for an ablation aperture, allowing for a more intense molecular beam. We use this nozzle to prepare a molecular beam of aluminum monohydride (AlH) suitable for ion trap loading of AlH$^+$ via photoionization in ultra-high vacuum. We demonstrate stable AlH production over hour time scales using a liquid ablation target. The long-term stability, low heat load and fast ion production rate of this source are well-suited to molecular ion experiments employing destructive state readout schemes requiring frequent trap reloading.

  11. Excimer laser-ablated plasma atomic spectrometry

    International Nuclear Information System (INIS)

    The characterization and evaluation of a new kind of excimer laser-ablated plasma and applications for direct spectrochemical analysis were investigated through time- and space-resolved spectroscopy. The shape, size, emission spectra, and excitation temperatures of the plasma are largely department on the atmospheric surroundings, the ambient gas composition, the pressure, and laser energy. Spatial discrimination may be desirable to increase the line-to-background (L/B) ratio in atomic emission spectroscopy. A direct spectrochemical analytical method for solid samples with good linearity was developed using the excimer laser-AES. The sensitivity of the analytical signal varied depending on the chemical matrix of the solid samples. A typical detection limit for potassium in a glass matrix was 0.13 μg/g.

  12. GHz Rabi flopping to Rydberg states in hot atomic vapor cells

    CERN Document Server

    Huber, B; Schlagmüller, M; Kölle, A; Kübler, H; Löw, R; Pfau, T

    2011-01-01

    We report on the observation of Rabi oscillations to a Rydberg state on a timescale below one nanosecond in thermal rubidium vapor. We use a bandwidth-limited pulsed excitation and observe up to 6 full Rabi cycles within a pulse duration of ~ 4 ns. We find good agreement between the experiment and numerical simulations based on a surprisingly simple model. This result shows that fully coherent dynamics with Rydberg states can be achieved even in thermal atomic vapor thus suggesting small vapor cells as a platform for room temperature quantum devices. Furthermore the result implies that previous coherent dynamics in single atom Rydberg gates can be accelerated by three orders of magnitude.

  13. Secondary laser cooling of strontium-88 atoms

    Energy Technology Data Exchange (ETDEWEB)

    Strelkin, S. A.; Khabarova, K. Yu., E-mail: kseniakhabarova@gmail.com; Galyshev, A. A.; Berdasov, O. I.; Gribov, A. Yu.; Kolachevsky, N. N.; Slyusarev, S. N. [Federal State Unitary Enterprise “All-Russia Research Institute for Physicotechnical and Radio Engineering Measurements” (VNIIFTRI) (Russian Federation)

    2015-07-15

    The secondary laser cooling of a cloud of strontium-88 atoms on the {sup 1}S{sub 0}–{sup 3}P{sub 1} (689 nm) intercombination transition captured into a magneto-optical trap has been demonstrated. We describe in detail the recapture of atoms from the primary trap operating on the strong {sup 1}S{sub 0}–{sup 1}P{sub 1} (461 nm) transition and determine the recapture coefficient κ, the number of atoms, and their temperature in the secondary trap as a function of experimental parameters. A temperature of 2 µK has been reached in the secondary trap at the recapture coefficient κ = 6%, which confirms the secondary cooling efficiency and is sufficient to perform metrological measurements of the {sup 1}S{sub 0}–{sup 3}P{sub 1} (698 nm) clock transition in an optical lattice.

  14. Supersonic pulsed free-jet of atoms and molecules of refractory metals: laser induced fluorescence spectroscopic studies on zirconium atoms and zirconium oxide molecules

    International Nuclear Information System (INIS)

    The experimental setup for generating supersonic pulsed free-jet containing atoms and molecules of refractory nature has been built. The technique of laser vaporization in conjunction with supersonic cooling is used to generate these species. The cooled atoms and molecules in supersonic free-jet are probed by laser induced fluorescence spectroscopy. In particular, the technique has been used to perform low-resolution laser induced fluorescence spectroscopy, limited by laser linewidth, on cold Zr atoms and ZrO molecules. The translational temperatures of ∼ 26.5 K and the rotational temperatures of ∼ 81 K have been achieved. It is possible to achieve the Doppler width of few tens of MHz allowing it to perform high-resolution spectroscopy on these atomic and molecular species. Also because of low rotational temperature of molecules the spectral congestion is greatly reduced. In general, this technique can be applied to perform spectroscopy on atoms and molecules of refractory nature. (author)

  15. Design for a compact CW atom laser

    Science.gov (United States)

    Power, Erik; Raithel, Georg

    2011-05-01

    We present a design for a compact continuous-wave atom laser on a chip. A 2D spiral-shaped quadrupole guide is formed by two 0.5 mm × 0.5 mm wires carrying 5 A each embedded in a Si wafer; a 1.5 mm × 0.5 mm wire on the bottom layer carries -10 A, producing a horizontal B-field that pushes the guiding channel center above the chip surface. The center-to-center separation between the top wires is varied from 1.6 mm at the start of the guide to 1 mm at the end, decreasing the guide height from ~ 500 μm to ~ 25 μm above the surface as the atoms travel the 70 cm-long guide. The magnetic gradient of the guiding channel gradually increases from ~ 100 G /cm to ~ 930 G /cm . These features result in continuous surface adsorption evaporative cooling and progressive magnetic compression. Spin flip losses are mitigated by a solenoid sewn around the guide to produce a longitudinal B-field. 87Rb atoms are gravitationally loaded into the guide. A far off-resonant light shift barrier at the end of the guide traps the atoms and allows formation of a BEC. Tuning the barrier height to create a non-zero tunneling rate equal to the loading rate completes the implementation of a CW atom laser. Two options for atom interferometry are implemented on the first-generation chip (matter-wave Fabry-Perot interferometer and guide-based Mach-Zehnder interferometer). Current construction status and challenges will be discussed, along with preliminary results.

  16. Dressed Gain from the Parametrically Amplified Four-Wave Mixing Process in an Atomic Vapor

    Science.gov (United States)

    Zhang, Zhaoyang; Wen, Feng; Che, Junling; Zhang, Dan; Li, Changbiao; Zhang, Yanpeng; Xiao, Min

    2015-10-01

    With a forward cone emitting from the strong pump laser in a thermal rubidium atomic vapor, we investigate the non-degenerate parametrically amplified four-wave mixing (PA-FWM) process with dressing effects in a three-level “double-Λ” configuration both theoretically and experimentally. By seeding a weak probe field into the Stokes or anti-Stokes channel of the FWM, the gain processes are generated in the bright twin beams which are called conjugate and probe beams, respectively. However, the strong dressing effect of the pump beam will dramatically affect the gain factors both in the probe and conjugate channels, and can inevitably impose an influence on the quantum effects such as entangled degree and the quantum noise reduction between the two channels. We systematically investigate the intensity evolution of the dressed gain processes by manipulating the atomic density, the Rabi frequency and the frequency detuning. Such dressing effects are also visually evidenced by the observation of Autler-Townes splitting of the gain peaks. The investigation can contribute to the development of quantum information processing and quantum communications.

  17. Coherent manipulation of atoms using laser light

    International Nuclear Information System (INIS)

    The internal structure of a particle an atom or other quantum system in which the excitation energies are discrete undergoes change when exposed to pulses of near-resonant laser light. This tutorial review presents basic concepts of quantum states, of laser radiation and of the Hilbert-space state vector that provides the theoretical portrait of probability amplitudes the tools for quantifying quantum properties not only of individual atoms and molecules but also of artificial atoms and other quantum systems. It discusses the equations of motion that describe the laser-induced changes (coherent excitation), and gives examples of laser=pulse effects, with particular emphasis on two-state and three-state adiabatic time evolution within the rotating-wave approximation. It provides pictorial descriptions of excitation based on the Bloch equations that allow visualization of two-state excitation as motion of a three-dimensional vector (the Bloch vector). Other visualization techniques allow portrayal of more elaborate systems, particularly the Hilbert-space motion of adiabatic states subject to various pulse sequences. Various more general multilevel systems receive treatment that includes degeneracies, chains and loop linkages. The concluding sections discuss techniques for creating arbitrary pre-assigned quantum states, for manipulating them into alternative coherent superpositions and for analyzing an unknown superposition. Appendices review some basic mathematical concepts and provide further details of the theoretical formalism, including photons, pulse propagation, statistical averages, analytic solutions to the equations of motion, exact solutions of periodic Hamiltonians, and population-trapping 'dark' states. (author)

  18. Selenium determination in biological material by atomic absorption spectrophotometry in graphite furnace and using vapor generation

    International Nuclear Information System (INIS)

    The applicability of the atomic absorption spectrophotometry to the determination of selenium in biological material using vapor generation and electrothermal atomization in the graphite furnace was investigated. Instrumental parameters and the analytical conditions of the methods were studied. Decomposition methods for the samples were tested, and the combustion in the Wickbold apparatus was chosen. (author)

  19. Instantaneous Measurement of Local Concentration and Vapor Fraction in Liquid-Gas Mixtures by Laser-Induced Breakdown Spectroscopy

    Science.gov (United States)

    Kido, Akihiro; Hoshi, Kenji; Kusaka, Hiroto; Ogawa, Hideyuki; Miyamoto, Noboru

    Laser-induced breakdown spectroscopy (LIBS) with atomic emission excited with a focused high-energy ND: YAG laser was applied to quantify the concentration and the vapor fraction of liquid-gas mixtures. With LIBS it is possible to quantify local concentrations accurately even in liquid-gas mixtures as the ratio of the number of fuel-borne hydrogen atoms to nitrogen or oxygen atoms in the ambient gas. The ratio has a strong linear relation with the ratio of the peak emission intensities regardless of phase of the fuel. As the full width at half maximum (FWHM) of the emission peak from the fuel-borne hydrogen increases linearly with the liquid fraction due to the Doppler shift with micro-explosions, the FWHM yields the fuel vapor fraction. Simultaneous, high-resolution measurements of equivalence ratios and vapor fractions in an intermittent fuel spray in a pressurized atmosphere were obtained with this method. The results showed that the tip of the intermittent spray has a richer mixture with a lower vapor fraction.

  20. Gravitational Wave Detection with Single-Laser Atom Interferometers

    Science.gov (United States)

    Yu, Nan; Tinto, Massimo

    2011-01-01

    A new design for a broadband detector of gravitational radiation relies on two atom interferometers separated by a distance L. In this scheme, only one arm and one laser are used for operating the two atom interferometers. The innovation here involves the fact that the atoms in the atom interferometers are not only considered as perfect test masses, but also as highly stable clocks. Atomic coherence is intrinsically stable, and can be many orders of magnitude more stable than a laser.

  1. Atom interferometric gravitational wave detection using heterodyne laser links

    CERN Document Server

    Hogan, Jason M

    2015-01-01

    We propose a scheme based on a heterodyne laser link that allows for long baseline gravitational wave detection using atom interferometry. While the baseline length in previous atom-based proposals is constrained by the need for a reference laser to remain collimated as it propagates between two satellites, here we circumvent this requirement by employing a strong local oscillator laser near each atom ensemble that is phase locked to the reference laser beam. Longer baselines offer a number of potential advantages, including enhanced sensitivity, simplified atom optics, and reduced atomic source flux requirements.

  2. Industrial aspects of precision machining with copper vapor lasers

    Science.gov (United States)

    Hartmann, Martin; Koch, Juergen; Lang, Adolf; Schutte, Karsten; Bergmann, Hans W.

    1997-08-01

    The applications of conventional infrared lasers running cw or quasi-sw for drilling, cutting and shaping are limited in the precision achievable due to the long interaction time which leads to heat affected zones. The necessity to use a gas jet to blow the molten material out of the cut kerf will damage fragile workpieces like thin foils. Short laser pulses of sufficient intensity remove the material directly by evaporation and minimize the amount of heat transferred into the solid. Classical infrared laser sources generate a shielding air plasma within some ns at power densities above some 107W/cm2. The optical breakdown threshold value in air can be shifted to higher intensities by using visible light as well as reducing the focal diameter. An alternative way is to shorten the pulse duration to less than 10 ps that a plasma is generated only after the pulse. Thus, the material removal process begins after the deposition of the pulse energy into the material. But such short pulses will generate a pressure wave due to the sudden thermal expansion and can damage or destroy microscopic components. For industrial production the productivity is a further aspect. Hence, a certain mean power is required in order to obtain the desired production rate. Considering the above aspects, copper vapor lasers (CVLs) with ns pulse duration are well suited for precision machining of metals and ceramics. Processing with CVLs is an advantage in that its wavelength is highly absorbed by metallic targets and the probability for the optical breakdown in air is low. CVLs in an oscillator-amplifier-setup incorporate diffraction limited beam quality and high average power. The present paper outlines the potential of the CVL for the industrial use regarding high processing speed and precision. Under these aspects the limiting mechanisms on the material removal process and the necessary processing strategies for scaling up the productivity are shown. The relevant laser parameters for

  3. Mathematical modeling of copper vapor laser and using it as a pumping source of dye laser

    International Nuclear Information System (INIS)

    A simple 'zero-dimensional' self-consistent mathematical model describing the discharge kinetics and lasing characteristics of copper and copper bromide vapor lasers with neon and hydrogen additives has been developed. The suggested model offers simple mechanisms to explain discharge kinetics mechanisms, different physical processes and hydrogen additive effects on CVL and Cu Br lasers. The model estimates the temporal evolution of discharge voltage and current, population densities, laser beam density, electron temperature and radial distribution of pressure, buffer gas temperature and the influence of the skin effect. (author)

  4. Laser Spectroscopy of Muonic Atoms and Ions

    CERN Document Server

    Pohl, Randolf; Fernandes, Luis M P; Ahmed, Marwan Abdou; Amaro, Fernando D; Amaro, Pedro; Biraben, François; Cardoso, João M R; Covita, Daniel S; Dax, Andreas; Dhawan, Satish; Diepold, Marc; Franke, Beatrice; Galtier, Sandrine; Giesen, Adolf; Gouvea, Andrea L; Götzfried, Johannes; Graf, Thomas; Hänsch, Theodor W; Hildebrandt, Malte; Indelicato, Paul; Julien, Lucile; Kirch, Klaus; Knecht, Andreas; Knowles, Paul; Kottmann, Franz; Krauth, Julian J; Bigot, Eric-Olivier Le; Liu, Yi-Wei; Lopes, José A M; Ludhova, Livia; Machado, Jorge; Monteiro, Cristina M B; Mulhauser, Françoise; Nebel, Tobias; Rabinowitz, Paul; Santos, Joaquim M F dos; Santos, José Paulo; Schaller, Lukas A; Schuhmann, Karsten; Schwob, Catherine; Szabo, Csilla I; Taqqu, David; Veloso, João F C A; Voss, Andreas; Weichelt, Birgit; Antognini, Aldo

    2016-01-01

    Laser spectroscopy of the Lamb shift (2S-2P energy difference) in light muonic atoms or ions, in which one negative muon $\\mu^-$ is bound to a nucleus, has been performed. The measurements yield significantly improved values of the root-mean-square charge radii of the nuclei, owing to the large muon mass, which results in a vastly increased muon wave function overlap with the nucleus. The values of the proton and deuteron radii are 10 and 3 times more accurate than the respective CODATA values, but 7 standard deviations smaller. Data on muonic helium-3 and -4 ions is being analyzed and will give new insights. In future, the (magnetic) Zemach radii of the proton and the helium-3 nuclei will be determined from laser spectroscopy of the 1S hyperfine splittings, and the Lamb shifts of muonic Li, Be and B can be used to improve the respective charge radii.

  5. Storage and Retrieval of Thermal Light in Warm Atomic Vapor

    OpenAIRE

    Cho, Young-Wook; Kim, Yoon-Ho

    2009-01-01

    We report slowed propagation and storage and retrieval of thermal light in warm rubidium vapor using the effect of electromagnetically-induced transparency (EIT). We first demonstrate slowed-propagation of the probe thermal light beam through an EIT medium by measuring the second-order correlation function of the light field using the Hanbury-Brown$-$Twiss interferometer. We also report an experimental study on the effect of the EIT slow-light medium on the temporal coherence of thermal light...

  6. [Vaporization of urethral stenosis using the KTP 532 laser].

    Science.gov (United States)

    Schmidlin, F; Oswald, M; Iselin, C; Rohner, S; Jichlinski, P; Delacrétaz, G; Leisinger, H J; Graber, P

    1997-01-01

    The authors treated 16 patients presenting with a total of 20 anterior urethral strictures using the KTP 16 Laser. The aetiology was iatrogenic in 50% of cases, infectious in 20% of cases, traumatic in 20% of cases and unknown in 10% of cases. The stricture was situated in the bulbous urethra (80%), membranous urethra (10%) or penil urethra (10%). Laser vaporization of the urethral stricture was performed over the entire circumference of the urethra when necessary, followed by bladder drainage by urethral catheter for 24 hours. All patients were prospectively reviewed at 3 weeks, 3 months and 6 months (clinical symptoms, uroflowmetry, cystourethrography). A complete symptom and urodynamic success was obtained in 13 patients (81%) at 3 and 6 months. The stricture recurred in 4 patients, but only three of them (19%) required treatment (reoperation of repeat dilatations). The mean maximum flow rate increased from 6 mL/s to 20 mL/s at 3 months and was maintained at 19 mL/s at 6 months. No intraoperative or postoperative complications were observed. In conclusion, our results confirm that KTP 532 laser urethral strictures is a reliable and effective method in the medium term. These good results also suggest an advantage in terms of the recurrence rate in comparison with internal urethrotomy. However, our series needs to be evaluated with a longer follow-up and prospective, randomized trials comparing the two methods need to be conducted. PMID:9157820

  7. Atomic mercury vapor inside a hollow-core photonic crystal fiber

    CERN Document Server

    Vogl, Ulrich; Joly, Nicolas Y; Russell, Philip St J; Marquardt, Christoph; Leuchs, Gerd

    2014-01-01

    We demonstrate high atomic mercury vapor pressure in a kagom\\'e-style hollow-core photonic crystal fiber at room temperature. After a few days of exposure to mercury vapor the fiber is homogeneously filled and the optical depth achieved remains constant. With incoherent optical pumping from the ground state we achieve an optical depth of 114 at the $6^3P_2 - 6^3D_3$ transition, corresponding to an atomic mercury number density of $6 \\times 10^{10}$ cm$^{-3}$. The use of mercury vapor in quasi one-dimensional confinement may be advantageous compared to chemically more active alkali vapor, while offering strong optical nonlinearities in the ultraviolet region of the optical spectrum.

  8. Research and development prospects for the atomic uranium laser isotope separation process. Research report 442

    International Nuclear Information System (INIS)

    Research and development activities are being conducted on many aspects of the atomic uranium laser isotope separation process. Extensive laser spectroscopy studies have been made in order to identify attractive multi-step selective ionization schemes. Using low density (1010 atoms/cm3) apparatus, the excited state spectra of atomic uranium have been investigated via multiple step laser excitation and photoionization studies using two, three and four pulsed lasers. Observation of the spectra was accomplished by observing the yield of 235U and 238U ions as a function of the wavelength, intensities and delays of the various lasers. These data yielded information on the photoexcitation and photoionizatin cross sections, and on the location, J values, lifetimes, isotope shifts and hyperfine structure of the various atomic levels of uranium. Experiments on selective ionization of uranium vapor by multiple step laser excitation followed by ion extraction at 1013 atoms/cm3 density have produced 6% enriched 235U. These indicate that this process is well adapted to produce light water reactor fuel but less suitable for highly enriched material. Application has been made for license for a 1979 experimental facility to provide data for a mid-1980 commercial plant

  9. Measuring the quantum statistics of an atom laser beam

    OpenAIRE

    Bradley, A. S.; Olsen, M. K.; Haine, S. A.; Hope, J. J.

    2006-01-01

    We propose and analyse a scheme for measuring the quadrature statistics of an atom laser beam using extant optical homodyning and Raman atom laser techniques. Reversal of the normal Raman atom laser outcoupling scheme is used to map the quantum statistics of an incoupled beam to an optical probe beam. A multimode model of the spatial propagation dynamics shows that the Raman incoupler gives a clear signal of de Broglie wave quadrature squeezing for both pulsed and continuous inputs. Finally, ...

  10. Endoscopic photodynamic therapy of tumors using gold vapor laser

    Science.gov (United States)

    Kuvshinov, Yury P.; Poddubny, Boris K.; Mironov, Andrei F.; Ponomarev, Igor V.; Shental, V. V.; Vaganov, Yu. E.; Kondratjeva, T. T.; Trofimova, E. V.

    1996-01-01

    Compact sealed-off gold vapor laser (GVL) with 2 W average power and 628 nm wavelength was used for endoscopic photodynamic therapy in 20 patients with different tumors in respiratory system and upper gastrointestinal tract. Russian-made hematoporphyrin derivative (Hpd) `Photohem' was used as a photosensitizer. It was given intravenously at a dose of 2 - 2.5 mg/kg body weight 48 hours prior to tumor illumination with 628 nm light from GVL. Intermittent irradiation with GVL was done through flexible endoscope always under local anaesthesia at a power of 200 - 400 mW/sm2 and a dose of 150 - 400 J/sm2. 80% patients showed complete or partial response depending on stage of tumor. In cases of early gastric cancer all patients had complete remission with repeated negative biopsies. No major complication occurred.

  11. Ion generation by laser and its application to metal vapor laser

    International Nuclear Information System (INIS)

    The phenomena of ion generation from laser-heated metallic targets are studied. The interest of this experiment is to know quantitatively the number of ions from targets with various elements and at the various stages of laser power. The pressure change in vacuum in the instance of plasma production is another important phenomenon. An application of laser plasma to the metal vapor ion-laser is considered. The experimental set-up is shown. The amount of ions and the energy were measured with a time-of-flight ion collector. The energy spectra of ions were analyzed with an electrostatic deflector. The pressure change in vacuum was measured with a vacuum gauge and a quadrupole mass filter. For ion generation, three different lasers were used. A flash-lamp pumped dye laser with rhodamine-6G emitted the energy up to 1 joule at wavelength of about 0.6 μm. Two TEA type CO2 lasers emitted the energy up to 1 joule and 15 joule at 10.6 μm with the pulse width of 80 ns and 0.3 μs. The time integrated ion current from Cd and Cu targets heated by the rhodamine-6G dye laser was measured as a function of laser energy. The Cd ion-laser oscillation by laser-produced plasma was observed. The intensity of radiation at the wavelength of 5378 A was measured as a function of the pumping CO2 laser power. The gain coefficient was about one order of magnitude as high as compared with electrical discharge-pumped He-Cd laser. (Kato, T.)

  12. Soliton Atom Laser with Quantum State Transfer Property

    Institute of Scientific and Technical Information of China (English)

    LIU Xiong-Jun; JING Hui; GE Mo-Lin

    2006-01-01

    @@ We study the nonlinear effects in the quantum states transfer technique from photons to matter waves in the three-level case, which may provide the formation of a soliton atom laser with nonclassical atoms. The validity of quantum transfer mechanism is confirmed in the presence of the intrinsic nonlinear atomic interactions. The accompanied frequency chirp effect is shown to have no influence on the grey solitons formed by the output atom laser and the possible quantum depletion effect is also briefly discussed.

  13. Atomic vapour laser isotope separation of zirconium

    International Nuclear Information System (INIS)

    The possibility of separating the 91Zr isotope from the rest of the isotopes of zirconium were investigated. The current interest in zirconium arise from the fact that zirconium is an important element in the construction of nuclear reactors. The technique proposed for the isotope separation process is different from those currently in use for the separation of isotopes of refractory elements such as uranium. The proposed isotope separation process is based on the multi-step selective excitation of the isotope to be extracted, which in this case is 91Zr. The isotope-selective laser excitation relies on the angular-momentum selection rules for the absorption of circularly polarized light. The theory governing the isotope separation process is discussed and the various parameters in the practical implementation of the theory are investigated. The suitability of a demountable hollow cathode lamp as zirconium atomic vapour source was investigated. The optimum working conditions for the demountable hollow cathode lamp was determined and fluorescence, absorption and emission measurements were made. In order to realize a selective two-step excitation process, relevant energy levels must exist which fulfill certain requirements as discussed in the thesis. Energy levels fulfilling the necessary conditions for isotope separation are not readily available and an intensive study of the zirconium energy levels were made. Non-selective two-step excitation of the zirconium atoms was realized. These fluorescence measurements gave information regarding the optical alignment of the laser beams as well as the construction of the demountable hollow cathode lamp as atomic vapour source for the two-step excitation process. Although selective two-step excitation of the 91Zr isotope could not be achieved, a number of valuable results were obtained during the project. Proposals on how the necessary selective excitation could be achieved, in order to realize the separation of the 91Zr

  14. [The physics of laser polarized muonic atoms

    International Nuclear Information System (INIS)

    This past research period we carried out a successful experiment at LAMPF in collaboration with Syracuse University in which we used lasers to produce polarized muonic 3He. Samples of nuclear polarized 3He were produced by spin-exchange with optically pumped rubidium vapor. Unpolarized muons were stopped in the gas, and became polarized due to their hyperfine interaction with the 3He nucleus. We determined that a muon polarization of ∼8% results with a 3He target polarization of 100%. The high statistical accuracy of our result gives us a firm handle on a theoretical question of great importance to future work involving muons and polarized 3He. Currently, we are working toward a new experiment at LAMPF, for which we have just submitted a proposal requesting running time this coming summer. The experiment utilizes a new technique for producing polarized muonic 3He, a technique we believe has the potential for producing practical polarizations that in principle could be as high as 75%, and in practice may exceed 25--50%. We call this new technique direct spin-exchange (DSE) because it is based on spin-exchange collisions between neutral muonic helium and an optically pumped vapor of Rb. It is direct because, in contrast to the technique we used last summer, the 3He nucleus is not involved in the spin-exchange process. We have proposed the use of DSE to study the induced pseudoscalar form factor of 3He. Finally, we describe an experiment to measure the spin dependent structure function of the neutron at SLAC. Princeton played an important role in the design and proposal of this experiment, including hosting a meeting to explore the technical feasibility of the polarized 3He target

  15. Collinear laser spectroscopy of atomic cadmium

    CERN Document Server

    Frömmgen, Nadja; Bissell, Mark L; Bieroń, Jacek; Blaum, Klaus; Cheal, Bradley; Flanagan, Kieran; Fritzsche, Stephan; Geppert, Christopher; Hammen, Michael; Kowalska, Magdalena; Kreim, Kim; Krieger, Andreas; Neugart, Rainer; Neyens, Gerda; Rajabali, Mustafa M; Nörtershäuser, Wilfried; Papuga, Jasna; Yordanov, Deyan T

    2015-01-01

    Hyperfine structure $A$ and $B$ factors of the atomic $5s\\,5p\\,\\; ^3\\rm{P}_2 \\rightarrow 5s\\,6s\\,\\; ^3\\rm{S}_1$ transition are determined from collinear laser spectroscopy data of $^{107-123}$Cd and $^{111m-123m}$Cd. Nuclear magnetic moments and electric quadrupole moments are extracted using reference dipole moments and calculated electric field gradients, respectively. The hyperfine structure anomaly for isotopes with $s_{1/2}$ and $d_{5/2}$ nuclear ground states and isomeric $h_{11/2}$ states is evaluated and a linear relationship is observed for all nuclear states except $s_{1/2}$. This corresponds to the Moskowitz-Lombardi rule that was established in the mercury region of the nuclear chart but in the case of cadmium the slope is distinctively smaller than for mercury. In total four atomic and ionic levels were analyzed and all of them exhibit a similar behaviour. The electric field gradient for the atomic $5s\\,5p\\,\\; ^3\\mathrm{P}_2$ level is derived from multi-configuration Dirac-Hartree-Fock calculatio...

  16. Gas lasers applied atomic collision physics, v.3

    CERN Document Server

    McDaniel, E W

    1982-01-01

    Applied Atomic Collision Physics, Volume 3: Gas Lasers describes the applications of atomic collision physics in the development of many types of gas lasers. Topics covered range from negative ion formation in gas lasers to high-pressure ion kinetics and relaxation of molecules exchanging vibrational energy. Ion-ion recombination in high-pressure plasmas is also discussed, along with electron-ion recombination in gas lasers and collision processes in chemical lasers.Comprised of 14 chapters, this volume begins with a historical summary of gas laser developments and an overview of the basic ope

  17. Ultrathin atomic vapor film transmission spectroscopy: analysis of Dicke narrowing structure

    Science.gov (United States)

    Li, Yuanyuan; Zhang, Yanpeng; Gan, Chenli

    2005-11-01

    Transmission sub-Doppler spectroscopy with confined atomic vapor film between two dielectric walls is theoretically studied. Because of atoms flying from wall to wall, where they get de-excited, the atom-field interaction time is anisotropic so that the contribution of slow atoms is enhanced, a sub-Doppler transmission spectroscopy (Dicke narrowing effect) can be obtained when the thickness of the film is much small or comparable with the wavelength even at small angle oblique incidence. It is feasible to get a sub-Doppler structure in a new region (L < ?/4) in experiments.

  18. Narrow linewidth single laser source system for onboard atom interferometry

    CERN Document Server

    Theron, Fabien; Renon, Geoffrey; Bidel, Yannick; Zahzam, Nassim; Cadoret, Malo; Bresson, Alexandre

    2014-01-01

    We present an original compact and robust laser system for atom interferometry based on a frequency-doubled telecom laser. Thanks to an original stabilization architecture on a saturated absorption, we obtain a frequency agile laser system allowing fast tuning of the laser frequency over 1 GHz in few ms using only a single laser source. The different laser frequencies used for atom interferometry are created by changing dynamically the frequency of the laser and by creating sidebands using a phase modulator. We take advantage of the maturity of fiber telecom technology to reduce the number of free-space optical components, which are intrinsically less stable, and to make the setup compact, much less sensitive to vibrations and thermal fluctuations. This source provides spectral linewidth below 2.5 kHz required for precision atom interferometry, and particularly for an high performance atomic inertial sensor.

  19. Laser vaporization of extravasation type of mucocele of the lower lip with 940-nm diode laser

    Directory of Open Access Journals (Sweden)

    G Agarwal

    2013-01-01

    Full Text Available A 43-year-old male presented with an asymptomatic swelling of the lower labial mucosa. Examination revealed that the tip of maxillary canine was causing trauma on the affected side. A diagnosis of extravasation type of mucocele was established clinically. Vaporization of the mucocele was done with a 940-nm diode laser in contact mode. The lesion healed uneventfully and there has been no recurrence for 3 months.

  20. Laser fluorescence spectroscopy of sputtered uranium atoms

    International Nuclear Information System (INIS)

    Laser induced fluorescence (LIF) spectroscopy was used to study the sputtering of 99.8% 238U metal foil when bombarded by normally incident 500 to 3000 eV Ne+, Ar+, Kr+, and O2+. A three-level atom model of the LIF processes is developed to interpret the observed fluorescent emission from the sputtered species. The model shows that close attention must be paid to the conditions under which the experiment is carried out as well as to the details of the collision cascade theory of sputtering. Rigorous analysis shows that when properly applied, LIF can be used to investigate the predictions of sputtering theory as regards energy distributions of sputtered particles and for the determination of sputtering yields. The possibility that thermal emission may occur during sputtering can also be tested using the proposed model. It is shown that the velocity distribution (either the number density or flux density distribution, depending upon the experimental conditions) of the sputtered particles can be determined using the LIF technique and that this information can be used to obtain a description of the basic sputtering mechanisms. These matters are discussed using the U-atom fluorescence measurements as a basis. The relative sputtering yields for various incident ions on uranium were also measured for the first time using the LIF technique. A surprisingly high fraction of the sputtered uranium atoms were found to occupy the low lying metastable energy levels of U(I). The population of the sputtered metastable atoms were found approximately to obey a Boltzman distribution with an effective temperature of 920 +- 1000K. 41 references

  1. Study of Rb - vapor coated cell; atomic diffusion and cell curing process

    CERN Document Server

    Atutov, S N; Plekhanov, A I; Sorokin, V A

    2015-01-01

    We present the results of the study of an optical resonant cell filled by a vapor of the Rb atoms and coated with a non-stick polydimethylsiloxane (PDMS) polymer. We show that it is possible to define correctly the diffusion coefficient of the atoms in the coating, using geometric parameters of the cell and the vapor density in the cell volume only. The dependence of the diffusion coefficient on the cell curing time is presented. It is shown that the mysterious cell curing process can be explained in terms of the polymerization of the polymer coating by alkali atoms. Anomalous long dwell time of the Rb atoms on the PDMS coating is discussed as well.

  2. Study of elimination of vapor atom deposition. Final report

    International Nuclear Information System (INIS)

    The major objective of this study was to define and evaluate methods by which an optical system could be protected from performance degradation arising from exposure to a beam of heavy metal atoms. The optical system is coupled to a chamber in which the metal atoms are being produced and processed. The coupling aperture is the source of the contaminating metal atom beam, which, if un-attenuated, would degrade the system performance in an unacceptably short period of time. It was agreed early in the program to concentrate on a gaseous scattering technique, with a stated objective of metal beam flux reduction of about 106. Additional constraints require that the scattering gas must not effuse back into the main process chamber at such a rate that it has significant effect on the vacuum level in the chamber, which is of the order of 10-6 torr; finally, the path length between the main chamber and the optical system must not be increased unduly. This report summarizes the analyses that were performed under the program. Section 2 presents a summary review, while the details of the analyses are described in Section 3. Recommendations leading toward final system design are given in Section 4. Finally, an appendix contains a description and printout of a program that was developed and used to facilitate the evaluation of system performance parametrically. 6 refs., 9 figs

  3. Influence of Size Effects on Uptake of Impurity Atoms by Aerosol Nanoparticles Growing in Vapor Condensation

    OpenAIRE

    Levdansky, V.V.

    2014-01-01

    It is known that impurity atoms (molecules) in the main substance can affect its physicochemical properties. Semiconductor doping is paramount in micro- and nanoelectronics. In some cases nanoparticle doping is needed. Nanoparticle doping in the general case depends on the size of nanoparticles. Below we consider theoretically size effects in the uptake of impurity (dopant) atoms by the aerosol nanoparticle that grows in the supersaturated vapor.

  4. Atomic stabilization in superintense laser fields

    International Nuclear Information System (INIS)

    Atomic stabilization is a highlight of superintense laser-atom physics. A wealth of information has been gathered on it; established physical concepts have been revised in the process; points of contention have been debated. Recent technological breakthroughs are opening exciting perspectives of experimental study. With this in mind, we present a comprehensive overview of the phenomenon. We discuss the two forms of atomic stabilization identified theoretically. The first one, 'quasistationary (adiabatic) stabilization' (QS), refers to the limiting case of plane-wave monochromatic radiation. QS characterizes the fact that ionization rates, as calculated from single-state Floquet theory, decrease with intensity (possibly in an oscillatory manner) at high values of the field. We present predictions for QS from various forms of Floquet theory: high frequency (that has led to its discovery and offers the best physical insight), complex scaling, Sturmian, radiative close coupling and R-matrix. These predictions all agree quantitatively, and high-accuracy numerical results have been obtained for hydrogen. Predictions from non-Floquet theories are also discussed. Thereafter, we analyse the physical origin of QS. The alternative form of stabilization, 'dynamic stabilization' (DS), is presented next. This expresses the fact that the ionization probability at the end of a laser pulse of fixed shape and duration does not approach unity as the peak intensity is increased, but either starts decreasing with the intensity (possibly in an oscillatory manner), or flattens out at a value smaller than unity. We review the extensive research done on one-dimensional models, that has provided valuable insights into the phenomenon; two- and three-dimensional models are also considered. Full three-dimensional Coulomb calculations have encountered severe numerical handicaps in the past, and it is only recently that a comprehensive mapping of DS could be made for hydrogen. An adiabatic

  5. Unraveling the Solid-Liquid-Vapor Phase Transition Dynamics at the Atomic Level with Ultrafast X-Ray Absorption Near-Edge Spectroscopy

    International Nuclear Information System (INIS)

    X-ray absorption near-edge spectroscopy (XANES) is a powerful probe of electronic and atomic structures in various media, ranging from molecules to condensed matter. We show how ultrafast time resolution opens new possibilities to investigate highly nonequilibrium states of matter including phase transitions. Based on a tabletop laser-plasma ultrafast x-ray source, we have performed a time-resolved (∼3 ps) XANES experiment that reveals the evolution of an aluminum foil at the atomic level, when undergoing ultrafast laser heating and ablation. X-ray absorption spectra highlight an ultrafast transition from the crystalline solid to the disordered liquid followed by a progressive transition of the delocalized valence electronic structure (metal) down to localized atomic orbitals (nonmetal--vapor), as the average distance between atoms increases.

  6. Cold atom dynamics in crossed laser beam waveguides

    CERN Document Server

    Torrontegui, E; Ruschhaupt, A; Guéry-Odelin, D; Muga, J G

    2010-01-01

    We study the dynamics of neutral cold atoms in an $L$-shaped crossed-beam optical waveguide formed by two perpendicular red-detuned lasers of different intensities and a blue-detuned laser at the corner. Complemented with a vibrational cooling process this setting works as a one-way device or "atom diode".

  7. GHz Rabi Flopping to Rydberg States in Hot Atomic Vapor Cells

    International Nuclear Information System (INIS)

    We report on the observation of Rabi oscillations to a Rydberg state on a time scale below 1 ns in thermal rubidium vapor. We use a bandwidth-limited pulsed excitation and observe up to 6 full Rabi cycles within a pulse duration of ∼4 ns. We find good agreement between the experiment and numerical simulations based on a surprisingly simple model. This result shows that fully coherent dynamics with Rydberg states can be achieved even in thermal atomic vapor, thus suggesting small vapor cells as a platform for room-temperature quantum devices. Furthermore, the result implies that previous coherent dynamics in single-atom Rydberg gates can be accelerated by 3 orders of magnitude.

  8. Vapor generation – atomic spectrometric techniques. Expanding frontiers through specific-species preconcentration. A review

    Energy Technology Data Exchange (ETDEWEB)

    Gil, Raúl A.; Pacheco, Pablo H.; Cerutti, Soledad [Área de Química Analítica, Facultad de Química Bioquímica y Farmacia, Universidad Nacional de San Luis, Ciudad de San Luis 5700 (Argentina); Instituto de Química de San Luis, INQUISAL, Centro Científico-Tecnológico de San Luis (CCT-San Luis), Consejo Nacional de Investigaciones Científicas y Universidad Nacional de San Luis, Ciudad de San Luis 5700 (Argentina); Martinez, Luis D., E-mail: ldm@unsl.edu.ar [Área de Química Analítica, Facultad de Química Bioquímica y Farmacia, Universidad Nacional de San Luis, Ciudad de San Luis 5700 (Argentina); Instituto de Química de San Luis, INQUISAL, Centro Científico-Tecnológico de San Luis (CCT-San Luis), Consejo Nacional de Investigaciones Científicas y Universidad Nacional de San Luis, Ciudad de San Luis 5700 (Argentina)

    2015-05-22

    This article reviews 120 articles found in SCOPUS and specific Journal cites corresponding to the terms ‘preconcentration’; ‘speciation’; ‘vapor generation techniques’ and ‘atomic spectrometry techniques’ in the last 5 years. - Highlights: • Recent advances in vapor generation and atomic spectrometry were reviewed. • Species-specific preconcentration strategies after and before VG were discussed. • New preconcentration and speciation analysis were evaluated within this framework. - Abstract: We review recent progress in preconcentration strategies associated to vapor generation techniques coupled to atomic spectrometric (VGT-AS) for specific chemical species detection. This discussion focuses on the central role of different preconcentration approaches, both before and after VG process. The former was based on the classical solid phase and liquid–liquid extraction procedures which, aided by automation and miniaturization strategies, have strengthened the role of VGT-AS in several research fields including environmental, clinical, and others. We then examine some of the new vapor trapping strategies (atom-trapping, hydride trapping, cryotrapping) that entail improvements in selectivity through interference elimination, but also they allow reaching ultra-low detection limits for a large number of chemical species generated in conventional VG systems, including complete separation of several species of the same element. This review covers more than 100 bibliographic references from 2009 up to date, found in SCOPUS database and in individual searches in specific journals. We finally conclude by giving some outlook on future directions of this field.

  9. A geração química de vapor em espectrometria atômica Chemical vapor generation in atomic spectrometry

    Directory of Open Access Journals (Sweden)

    Iracema Takase

    2002-12-01

    Full Text Available The historical development of atomic spectrometry techniques based on chemical vapor generation by both batch and flow injection sampling formats is presented. Detection via atomic absorption spectrometry (AAS, microwave induced plasma optical emission spectrometry (MIP-OES, inductively coupled plasma optical emission spectrometry (ICP-OES , inductively coupled plasma mass spectrometry (ICP-MS and furnace atomic nonthermal excitation spectrometry (FANES are considered. Hydride generation is separately considered in contrast to other methods of generation of volatile derivatives. Hg ¾ CVAAS (cold vapor atomic absorption spectrometry is not considered here. The current state-of-the-art, including extension, advantages and limitations of this approach is discussed.

  10. On the transverse mode of an atom laser

    OpenAIRE

    Busch, Th.; Köhl, M.; Esslinger, T.; Molmer, K.

    2001-01-01

    The transverse mode of an atom laser beam that is outcoupled from a Bose-Einstein condensate is investigated and is found to be strongly determined by the mean--field interaction of the laser beam with the condensate. Since for repulsive interactions the geometry of the coupling scheme resembles an interferometer in momentum space, the beam is found show filamentation. Observation of this effect would prove the transverse coherence of an atom laser beam.

  11. Multiphoton resonance ionization for hydrogen atom in laser field

    International Nuclear Information System (INIS)

    The Schroedinger equation of hydrogen atom in laser field is expanded by Floquet wave and can be solved by the iterative method. The atomic ionization by laser field is a complex eigenvalue problem, which is formed from differential equation and boundary condition. Then the formula of the multiphoton resonance ionization in a linear polarization laser field was obtained and it is compared with the experiment

  12. Electroionization lasers using electron transitions in inert gas atoms

    Science.gov (United States)

    Basov, N. G.; Danilychev, V. A.; Kholin, I. V.

    1986-04-01

    Recent developments in high-power quasi-continuous-wave lasers based on electron transitions in inert gas atoms and pumped by fast electrons or by the electroionization method are reviewed. In particular, attention is given to high-pressure lasers using atomic transitions in XeI, KrI, ArI, and NeI which generate in the visible and near-infrared regions of the spectrum. The advantages of these lasers over other high-power lasers and, particularly, over the CO2 laser are examined.

  13. Laser Methods in the Study of Nuclei, Atoms and Molecules

    Science.gov (United States)

    Inamura, Takashi T.

    2005-01-01

    The VIth International Workshop on Application of Lasers in Atomic Nuclei Research was held at Adam Mickiewicz University, Poznan in Poland from May 24 to 27, 2004. Its title this year was "Laser methods in the study of nuclei, atoms and molecules". Some topics are reviewed from a viewpoint of the atomic physics contribution to nuclear physics and its applications. It is suggested how this meeting should be organized in the future by taking the new geopolitics into account.

  14. Gravitational wave detection with single-laser atom interferometers

    OpenAIRE

    Yu, Nan; Tinto, Massimo

    2010-01-01

    We present a new general design approach of a broad-band detector of gravitational radiation that relies on two atom interferometers separated by a distance L. In this scheme, only one arm and one laser will be used for operating the two atom interferometers. We consider atoms in the atom interferometers not only as perfect inertial reference sensors, but also as highly stable clocks. Atomic coherence is intrinsically stable and can be many orders of magnitude more stable than a laser. The un...

  15. The linewidth of a non-Markovian atom laser

    OpenAIRE

    Hope, J. J.; Moy, G. M.; Collett, M. J.; Savage, C. M.

    1999-01-01

    We present a fully quantum mechanical treatment of a single mode atom laser including pumping and output coupling. By ignoring atom-atom interactions, we have solved this model without making the Born-Markov approximation. We find substantially less gain narrowing than is predicted under that approximation.

  16. Introduction to the theory of laser-atom interactions

    CERN Document Server

    Mittleman, Marvin H

    1993-01-01

    In response to the explosion of theories and experiments since the appearance of the first edition, the author has revised and expanded his basic text New sections include up-to-date discussions of multiphoton ionization, and electron-atom and atom-atom scattering in laser fields, reaffirming the work's position as the standard introduction to the field

  17. Light scattering studies of solids and atomic vapors

    Energy Technology Data Exchange (ETDEWEB)

    Chiang, T.C.

    1978-09-01

    The general technique of light scattering and luminescence was used to study the properties of a number of material systems. First, multi-phonon resonant Raman scattering up to four phonons in GaSe and one- and two-phonon resonant Raman scattering in the mixed GaS/sub x/Se/sub 1-x/ crystals with x < or = 0.23 were investigated. Second, the observation of one-phonon resonant Raman scattering in HfS/sub 2/ is reported. The result is used to determine the position of the direct gap of HfS/sub 2/. Third, the first observation of the ..pi..-polarized one-magnon luminescence sideband of the /sup 4/T/sub lg/ (/sup 4/G) ..-->.. /sup 6/A/sub lg/(/sup 6/S) excitonic transition in antiferromagnetic MnF/sub 2/ is presented. An effective temperature of the crystal is deduced from the simultaneously observed anti-Stokes sideband emission. Multi-magnon (< or = 7) excitonic luminescence sidebands were also observed in MnF/sub 2/, KMnF/sub 2/, and RbMnF/sub 3/ using pulsed excitation and detection. A simple model based on two-ion local exchange is proposed to explain the results qualitatively. Fourth, the first observation of two-magnon resonant Raman scattering in MnF/sub 2/ around the magnon sidebands is reported. A simple theoretical description explains the experimental observations. Fifth, a detailed theory of exciton-exciton interaction in MnF/sub 2/ is developed to explain and to predict the experimental results on two-exciton absorption, high level excitation, and exciton--exciton scattering. Sixth, Brillouin scattering was used to obtain the five independent elastic constants of the layered compound GaSe. The results show clear elastic anisotropy of the crystal. Resonant Brillouin scattering near the absorption edge was also studied, but no resonant enhancement was found. Seventh, two-photon parametric scattering in sodium vapor was studied. Phase matching angles and scattering cross sections are calculated for a given set of experimental conditions.

  18. Laser Cooling and Trapping of Neutral Mercury Atoms Using an Optically-Pumped External-Cavity Semiconductor Laser

    Science.gov (United States)

    Paul, Justin; Lytle, Christian; Jones, R. Jason

    2011-05-01

    The level structure of the Hg atom is similar to other alkaline earth-like atoms, offering the possibility to realize an extremely high quality resonance factor (Q) on the ``clock'' transition (1S0- 3P0) when confined in an optical lattice at the Stark-shift free wavelength. A key feature of the Hg system is the reduced uncertainty due to black-body induced Stark shifts, making it an interesting candidate as an optical frequency standard. One challenge to laser-cooling neutral Hg atoms is finding a reliable source for cooling on the 1S0-3 P1 transition at 253.7 nm. We employ an optically pumped semiconductor laser (OPSEL) operating at 1015 nm, whose frequency is quadrupled in two external-cavity doubling stages to generate over 120 mW at 253.7 nm. With this new laser source we have trapped Hg199 from a background vapor in a standard MOT. We trap up to 2 × 106 atoms with a 1/e2 radius of our MOT of ~310 microns, corresponding to a density of 1.28 × 1010 atoms/cm3. We report on the progress of our Hg system and plans for precision lattice-based spectroscopy of the clock transition. Support for this work is supported through the U.S. Air Force Office of Scientific Research (AFOSR) through grant no. FA9550-09-1-0563.

  19. Redistribution of light frequency by multiple scattering in a resonant atomic vapor

    CERN Document Server

    Carvalho, J C de A; Oriá, M; Chevrollier, M; de Silans, T Passerat

    2015-01-01

    The propagation of light in a resonant atomic vapor can \\textit{a priori} be thought of as a multiple scattering process, in which each scattering event redistributes both the direction and the frequency of the photons. Particularly, the frequency redistribution may result in L\\'evy flights of photons, directly affecting the transport properties of light in a resonant atomic vapor and turning this propagation into a superdifusion process. Here, we report on a Monte-Carlo simulation developed to study the evolution of the spectrum of the light in a resonant thermal vapor. We observe the gradual change of the spectrum and its convergence towards a regime of Complete Frequency Redistribution as the number of scattering events increases. We also analyse the probability density function of the step length of photons between emissions and reabsorptions in the vapor, which governs the statistics of the light diffusion. We observe two different regime in the light transport: superdiffusive when the vapor is excited n...

  20. Laser vaporization/ionization interface for coupling microscale separation techniques with mass spectrometry

    Science.gov (United States)

    Yeung, Edward S.; Chang, Yu-chen

    1999-06-29

    The present invention provides a laser-induced vaporization and ionization interface for directly coupling microscale separation processes to a mass spectrometer. Vaporization and ionization of the separated analytes are facilitated by the addition of a light-absorbing component to the separation buffer or solvent.

  1. Acetone vapor sensing using a vertical cavity surface emitting laser diode coated with polystyrene

    DEFF Research Database (Denmark)

    Ansbæk, Thor; Nielsen, Claus Højgaard; Larsen, Niels Bent;

    2009-01-01

    We report theoretical and experimental on a new vapor sensor, using a single-mode vertical-cavity surface-emitting laser (VCSEL) coated with a polymer sensor coating, which can detect acetone vapor at a volume fraction of 2.5%. The sensor provides the advantage of standard packaging, small form...

  2. Note: A novel and robust circuit for jitter reduction in copper vapor laser system

    Science.gov (United States)

    Mishra, R. K.; Raju, D. V. S.; Nakhe, S. V.

    2015-11-01

    A novel circuit scheme is presented to improve timing jitter performance of high voltage pulse power supply utilizing semiconductor switches and magnetic pulse compressors, for pumping pulsed copper vapor lasers. The circuit effectively handles reflected energy from the laser load and achieves better jitter performance. The proposed circuit scheme had typical jitter value of ±2 ns whereas the standard circuit used earlier had jitter of more than ±10 ns under similar conditions. Performance of the circuit scheme is studied on a copper vapor laser operating at average laser power of 40 W.

  3. Innershell X-ray laser in sodium vapor: Final steps towards Experimental verification

    Czech Academy of Sciences Publication Activity Database

    Nejdl, Jaroslav; Mocek, Tomáš; Rus, Bedřich; Sebban, S.; Wellegehausen, B.

    Dordrecht: Springer, 2009 - (Ciaran, L.; Riley, D.), S.557-562 ISBN 978-1-4020-9923-6. [International Conference on X-Ray Lasers /11th./. Belfast (GB), 17.08.2008-22.08.2008] R&D Projects: GA AV ČR KAN300100702 Institutional research plan: CEZ:AV0Z10100523 Keywords : inner-shell, X-ray laser, sodium vapor * x-ray laser * sodium vapor Subject RIV: BH - Optics, Masers, Lasers http://www.springer.com/physics/optics/book/978-1-4020-9923-6

  4. Optical pumping of rubidium atoms with tunable laser diodes

    International Nuclear Information System (INIS)

    A number of experiments on optical pumping of vapors of a mixture of rubidium isotopes is performed using diode lasers tunable in the vicinity of the D1-line. It is shown that the absorption spectrum of vapors changes drastically under laser irradiation tuned to certain components of the hyperfine structure of the D1-line. The absorption spectrum exhibits narrow peaks and holes related to the velocity-selective optical pumping and cross resonances. By using pulsed pumping across the magnetic field, Larmor oscillations of absorption are induced for a probe beam directed across the magnetic field

  5. Atomic vapour laser isotope separation in France

    International Nuclear Information System (INIS)

    France has a specific position in the uranium enrichment market. It has a major nuclear park, supplying 75% of the nation's electricity. On one hand the modern multinational EURODIF gaseous diffusion plant (10.8 M.SWU/y) works smoothly, and its supply of nuclear generated electricity offers customers a good long term view on enrichment costs. A program to improve its performances and to extend its lifespan is well in progress. It will offer a fast modulation capability, with advantage of off-peak power for about 3/4 of its electrical requirements. On the other hand, today's situation of over capacity, accentuated by non-commercial practices, may lead to a brutal restructuring of the world-wide enrichment industry in the coming years. The French approach has a long term goal, with a priority for a high performance process, which will be available when world stocks of enriched uranium are exhausted, and aging enrichment plants have to be shut down. To reach this goal, French Atomic Energy Commission has focused since 1985 on the atomic laser route, SILVA, in agreement with the industrial operator, COGEMA. Fully integrated pre-industrial experience, too costly, will be delayed as long as possible, toward the end of the decade. It will benefit from the most advanced options, taking into account the difficulty of changing them once demonstration has been achieved. The SILVA program is periodically assessed from both the scientific and the industrial point of view and a general assessment is to be made between 1996 and 1997, prior to pre-industrial development

  6. Temporal intensity correlation of light scattered by a hot atomic vapor

    CERN Document Server

    Dussaux, A; Guerin, W; Alibart, O; Tanzilli, S; Vakili, F; Kaiser, R

    2016-01-01

    We present temporal intensity correlation measurements of light scattered by a hot atomic vapor. Clear evidence of photon bunching is shown at very short time-scales (ns) imposed by the Doppler broadening of the hot vapor. Moreover, we demonstrate that some relevant information about the scattering process, such as the ratio of single to multiple scattering, can be deduced from the measured intensity correlation function. These measurements confirm the interest of temporal intensity correlation measurements to access non-trivial spectral features, with potential applications in astrophysics.

  7. Investigations of laser pumped gas cell atomic frequency standard

    Science.gov (United States)

    Volk, C. H.; Camparo, J. C.; Fueholz, R. P.

    1982-01-01

    The performance characteristics of a rubidium gas cell atomic frequency standard might be improved by replacing the standard rubidium discharge lamp with a single mode laser diode. Aspects of the laser pumped gas cell atomic clock studied include effects due to laser intensity, laser detuning, and the choice of the particular atomic absorption line. Results indicate that the performance of the gas cell clock may be improved by judicious choice of the operating parameters of the laser diode. The laser diode also proved to be a valuable tool in investigating the operation of the conventional gas cell clock. Results concerning linewidths, the light shift effect and the effect of isotopic spin exchange in the conventional gas cell clock are reported.

  8. Recent progress of laser cooling for neutral mercury atom

    Science.gov (United States)

    Liu, Kang-Kang; Zhao, Ru-Chen; Fu, Xiao-Hu; Hu, Jin-Meng; Feng, Yan; Xu, Zhen; Wang, Yu-Zhu

    2014-11-01

    Mercury is the heaviest stable atom that could be laser cooled, and have a large nuclear charge number. So it has a distinct advantage in quantum precision measurement such as fine-structure constant α and permanent electric dipole moment. Due to its insensitivity of black body radiation, atomic mercury is a good candidate of optical clock. Here we report our recent development of laser cooling of neutral mercury atom. By cooling the mercury source to about -70°C, an ultra-high vacuum system was realized to produce ultracold mercury atoms. The commercial frequency quadrupled semiconductor laser is locked on the cooling transition (1S0-3P1 transition, wavelength of 253.7 nm) by sub-Doppler frequency modulation spectroscopy. By the modification with feed-forward method, the UV laser becomes faster tunable and more stable. A folded beam configuration was used to realize the magneto-optical trap (MOT) because of the shortage of cooling laser power, and the ultracold mercury atoms were observed by fluorescence detection. All of six rich abundant isotopes have been observed, and the atom number is about 1.5×106 with density of 3.5×109 /cm3 for 202Hg. With optical shutter and the programmable system to control the time sequence, the temperature of ultracold atoms can be measured by time of flight method. To enhance the laser power, a 1014.8 nm fiber laser amplifier was developed, which can work at room temperature. After two stages of frequency doubling, about 75 mW of 253.7 nm UV laser were generated, and the saturated absorption spectroscopy of mercury atom was also observed. More power of UV laser could help to trap more atoms in the future. These works laid a good foundation to realize the mercury lattice clock.

  9. Comparison of the treatment of vascular lesions with the copper-vapor laser and flashlamp-pumped dye laser

    Science.gov (United States)

    Flock, Stephen T.; Waner, Milton; McGrew, Ben; Colvin, G. B.; Montague, Donna

    1992-08-01

    Vascular lesions such as port-wine stains and telangiectases are sometimes treated with carbon-dioxide lasers, argon lasers or argon-pumped dye lasers; however these lasers are non- specific in their thermal effect on tissues and as a result often cause significant scarring. Recently, evidence has accumulated that the flashlamp-pumped dye (585 nm) and copper- vapor (578 nm) lasers, which produce pulsed light that is efficiently absorbed by hemoglobin, are more selective in coagulating abnormal vascular tissue and as a result give a superior clinical result. It is not yet clear what the most important physical and biological mechanisms are during the light-tissue interaction mediated by these two lasers. The post-treatment sequence of events is different for tissue irradiated by each laser; most significantly, the flashlamp-pumped dye laser causes significant transient purpura, whereas the copper vapor laser causes blanching and eschar formation. The clinical outcome, that is regression of the lesion, is equally successful with either laser although some evidence has accumulated showing that the flashlamp-pumped dye laser is best suited to the treatment of small vessel disease while the copper-vapor laser is better for the treatment of large vessel disease. In this paper, we will discuss our observations of the treatment of vascular lesions on humans with the copper-vapor and flashlamp-pumped dye lasers using empirically derived efficacious treatment parameters. Mathematical models of light and heat propagation and in vivo experiments involving mice ears and rat skin flaps will be used to elucidate what we feel are the important underlying mechanisms of this vascular lesion laser therapy.

  10. Ionization characteristics of three-level atoms by nonmonochromatic lasers

    International Nuclear Information System (INIS)

    Ionization characteristics of two-step excitation by two intense nonmonochromatic (finite bandwidth) lasers are investigated. By approximating the laser fields by a stochastic model of a chaotic field, the stochastic atomic-density-matrix equations for three-level atoms are first obtained. Comparing with the analytical solution, the accuracy of our model is confirmed. By using this model, the ionization characteristics are studied in detail as a function of laser bandwidth. The dependence of laser bandwidth on the Doppler averaged ionization probability is also investigated. (author)

  11. Pulsed CO2 laser for intra-articular cartilage vaporization and subchondral bone perforation in horses

    Science.gov (United States)

    Nixon, Alan J.; Roth, Jerry E.; Krook, Lennart P.

    1991-05-01

    A pulsed carbon dioxide laser was used to vaporize articular cartilage in four horses, and perforate the cartilage and subchondral bone in four horses. Both intercarpal joints were examined arthroscopically and either a 1 cm cartilage crater or a series of holes was created in the third carpal bone of one joint. The contralateral carpus served as a control. The horses were evaluated clinically for 8 weeks, euthanatized and the joints examined radiographically, grossly, and histologically. Pulsed carbon dioxide laser vaporized cartilage readily but penetrated bone poorly. Cartilage vaporization resulted in no greater swelling, heat, pain on flexion, lameness, or synovial fluid reaction than the sham procedure. Laser drilling resulted in a shallow, charred hole with a tenacious carbon residue, and in combination with the thermal damage to deeper bone, resulted in increased swelling, mild lameness and a low-grade, but persistent synovitis. Cartilage removal by laser vaporization resulted in rapid regrowth with fibrous and fibrovascular tissue and occasional regions of fibrocartilage at week 8. The subchondral bone, synovial membrane, and draining lymph nodes appeared essentially unaffected by the laser cartilage vaporization procedure. Conversely, carbon dioxide laser drilling of subchondral bone resulted in poor penetration, extensive areas of thermal necrosis of bone, and significant secondary damage to the apposing articular surface of the radial carpal bone. The carbon dioxide laser is a useful intraarticular instrument for removal of cartilage and has potential application in inaccessible regions of diarthrodial joints. It does not penetrate bone sufficiently to have application in subchondral drilling.

  12. Vapor-melt Ratio in Laser Fine Cutting of Slot Arrays

    International Nuclear Information System (INIS)

    In order to improve cut quality for slot arrays, a new method of laser fine cutting under the consideration of the ratio of vapor to melt is presented. Laser cutting of 6063 aluminum alloy sheet, 0.5 mm in thickness, was carried out on a JK701H Nd:YAG pulse laser cutting system. The effects of vapor-melt ratio on kerf width, surface roughness and recast layer were studied which relate cutting qualities. Observation on the cut samples with different vapor-melt ratios (0.687, 1.574, 3.601 varied with laser power increasing, and 1.535, 3.601, 7.661 with decreasing of beam cutting speed) shows that high vapor-melt ratio improves laser cut quality clearly. Kerf width 0.2 mm of smooth area on kerf top area and thickness 2.03 μm of recast layer are obtained. No dross was found on the kerf bottom and the percentage of the smooth area is up to 40% out of whole kerf side. The research on vapor-melt ratio provides a deeper understanding of laser cutting and improves laser cut quality effectively.

  13. Advances in Diode-Laser-Based Water Vapor Differential Absorption Lidar

    Science.gov (United States)

    Spuler, Scott; Repasky, Kevin; Morley, Bruce; Moen, Drew; Weckwerth, Tammy; Hayman, Matt; Nehrir, Amin

    2016-06-01

    An advanced diode-laser-based water vapor differential absorption lidar (WV-DIAL) has been developed. The next generation design was built on the success of previous diode-laser-based prototypes and enables accurate measurement of water vapor closer to the ground surface, in rapidly changing atmospheric conditions, and in daytime cloudy conditions up to cloud base. The lidar provides up to 1 min resolution, 150 m range resolved measurements of water vapor in a broad range of atmospheric conditions. A description of the instrument and results from its initial field test in 2014 are discussed.

  14. Experiments with a laser cooled cloud of atoms

    OpenAIRE

    Natarajan, Vasant; Banerjee, Ayan; Rapol, Umakant

    1999-01-01

    We discuss two experiments that can be performed using a cloud of laser-cooled and trapped atoms, namely Bose-Einstein condensation (BEC) and search for a permanent Electric Dipole Moment (EDM). BEC can be observed in Rb atoms in a magnetic trap by using forced evaporative cooling to continuously lower the temperature below the condensation limit. The cloud is cooled by preferentially ejecting the hottest atoms from a magnetic trap. The magnetic trap is loaded with laser-cooled atoms from a m...

  15. Laser radiation effect on the mobility of iron atoms

    International Nuclear Information System (INIS)

    With the aid of radioactive isotopes the effect is studied of the radiation of a ruby laser on the mobility of iron atoms. In the region of interaction of the laser radiation with the specimen penetration is detected of isotope atoms to a depth greatly exceeding the heating zone. The mass transfer rate is determined, and a possible mechanism of the observed effect is considered. It is suggested that the substantial increase in atom mobility is due to the migration of interstitial atoms in the crystal lattice

  16. New niobium and rhenium halides synthesis routes by atomic vaporization. X-ray absorption spectroscopy characterization

    International Nuclear Information System (INIS)

    New synthetic route as the so called 'chimie douce' or MVS (Metal Vapor Synthesis) has been an increasing field lately to synthesize new kind of solid state structures. Our interest is the assembly of small molecular building blocks of early transition metal halides. We illustrate the use of vaporized rare earth metals to condense NbCls units. We probed the local order around the Nb atom with X-Ray Absorption Spectroscopy, far Infra-Red and XPS in order to better understand the mechanisms involved. A first EXAFS, IR and XPS study on solid state products has shown the evolution of the NbCl5 dimer towards a chain like structure. However, the condensation patterns depends on the rare earth atoms vaporized. These results have been confirmed by X-ray Absorption ab initio calculations. Because our compounds are extremely air sensitive we have developed in situ MVS reactor to take 'snapshots' of the structural intermediates by EXAFS. This study showed the condensation of the initial NbCl5 building blocks by reduction of the Nb oxidation state by rare earth vaporization. This method is a new way of looking at condensation mechanisms via structural evolution observed by EXAFS. (author)

  17. A geração química de vapor em espectrometria atômica Chemical vapor generation in atomic spectrometry

    OpenAIRE

    Iracema Takase; Hugo Borges Pereira; Aderval S. Luna; Patrícia Grinberg; Reinaldo Calixto de Campos

    2002-01-01

    The historical development of atomic spectrometry techniques based on chemical vapor generation by both batch and flow injection sampling formats is presented. Detection via atomic absorption spectrometry (AAS), microwave induced plasma optical emission spectrometry (MIP-OES), inductively coupled plasma optical emission spectrometry (ICP-OES) , inductively coupled plasma mass spectrometry (ICP-MS) and furnace atomic nonthermal excitation spectrometry (FANES) are considered. Hydride generation...

  18. Laser-enhanced ionization of mercury atoms in an inert atmosphere with avalanche amplification of the signal.

    Science.gov (United States)

    Clevenger, W L; Matveev, O I; Cabredo, S; Omenetto, N; Smith, B W; Winefordner, J D

    1997-07-01

    A new method for laser-enhanced ionization detection of mercury atoms in an inert gas atmosphere is described. The method, which is based on the avalanche amplification of the signal resulting from the ionization from a selected Rydberg level reached by a three-step laser excitation of mercury vapor in a simple quartz cell, can be applied to the determination of this element in various matrices by the use of conventional cold atomization techniques. The overall (collisional + photo) ionization efficiency is investigated at different temperatures, and the avalanche amplification effect is reported for Ar and P-10 gases at atmospheric pressure. It is shown that the amplified signal is related to the number of charges produced in the laser-irradiated volume. Under amplifier noise-limited conditions, a detection limit of ∼15 Hg atoms/laser pulse in the interaction region is estimated. PMID:21639354

  19. On a Mechanism for Limiting the Frequency and Energy Characteristics of Lasers on Self-terminating Transitions of Metal Atoms

    Science.gov (United States)

    Yudin, N. A.; Yudin, N. N.

    2016-04-01

    Electrophysical approach to estimation of conditions for efficient pumping of active medium of lasers on selfterminating transitions of metal atoms in a gas discharge tube with electrodes in cold buffer zones is used. Existence of processes that enhance the effect of the well-known mechanism of limitation of radiation frequency and energy characteristics caused by the presence of a pre-pulse electron concentration in the discharge circuit of lasers on self-terminating transitions of metal atoms is demonstrated. The mechanism of influence of these processes on frequency and energy characteristics of lasers on self-terminating transitions of metal atoms and the technical methods of neutralization of these processes are considered. It is shown that the practical efficiency of a copper vapor laser can attain ~10% under conditions of neutralization of these processes.

  20. Vacuum ultraviolet laser induced fluorescence on a Si atomic beam

    Science.gov (United States)

    O'Brian, T. R.; Lawler, J. E.

    1991-01-01

    A broadly applicable vacuum ultraviolet experiment is described for measuring radiative lifetimes of neutral and singly-ionized atoms in a beam environment to 5-percent accuracy using laser induced fluorescence. First results for neutral Si are reported.

  1. Laser Source for Atomic Gravity Wave Detector Project

    Data.gov (United States)

    National Aeronautics and Space Administration — Develop an Atom Interferometry-based gravity wave detector (vs Optical Interferometry). Characterize a high power laser. Use Goddard Space Flight Center Mission...

  2. Absorption spectroscopy characterization measurements of a laser-produced Na atomic beam

    Energy Technology Data Exchange (ETDEWEB)

    Ching, C.H.; Bailey, J.E.; Lake, P.W.; Filuk, A.B.; Adams, R.G.; McKenney, J.

    1996-06-01

    This work describes a pulsed Na atomic beam source developed for spectroscopic diagnosis of a high-power ion diode on the Particle Beam Fusion Accelerator II. The goal is to produce a {approximately} 10{sup 12}-cm{sup {minus}3}-density Na atomic beam that can be injected into the diode acceleration gap to measure electric and magnetic fields from the Stark and Zeeman effects through laser-induced-fluorescence or absorption spectroscopy. A {approximately} 10 ns fwhm, 1.06 {micro}m, 0.6 J/cm{sup 2} laser incident through a glass slide heats a Na-bearing thin film, creating a plasma that generates a sodium vapor plume. A {approximately} 1 {micro}sec fwhm dye laser beam tuned to 5,890 {angstrom} is used for absorption measurement of the Na I resonant doublet by viewing parallel to the film surface. The dye laser light is coupled through a fiber to a spectrograph with a time-integrated CCD camera. A two-dimensional mapping of the Na vapor density is obtained through absorption measurements at different spatial locations. Time-of-flight and Doppler broadening of the absorption with {approximately} 0.1 {angstrom} spectral resolution indicate that the Na neutral vapor temperature is about 0.5 to 2 eV. Laser-induced-fluorescence from {approximately} 1 {times} 10{sup 12}-cm{sup {minus}3} Na I 3s-3p lines observed with a streaked spectrograph provides a signal level sufficient for {approximately} 0.06 {angstrom} wavelength shift measurements in a mock-up of an ion diode experiment.

  3. Early Stages of the Chemical Vapor Deposition of Pyrolytic Carbon Investigated by Atomic Force Microscopy

    OpenAIRE

    Pfrang, Andreas; WAN Yong-Zhong; Schimmel, Thomas

    2009-01-01

    The early stages of chemical vapor deposition of pyrolytic carbon on planar silicon substrates were studied by the atomic force microscopy-based technique of chemical contrast imaging. Short deposition times were chosen to focus on the early stages of the deposition process, and three different types of nucleation were found: random nucleation of single islands, nucleation of carbon islands along lines and secondary nucleation which corresponds to the nucleation of carbon islands at the edges...

  4. Atomic characterization of Au clusters in vapor-liquid-solid grown silicon nanowires

    Energy Technology Data Exchange (ETDEWEB)

    Chen, Wanghua; Roca i Cabarrocas, Pere [Laboratoire de Physique des Interfaces et Couches Minces (LPICM), UMR 7647, CNRS, Ecole Polytechnique, 91128 Palaiseau (France); Pareige, Philippe; Castro, Celia [Groupe de Physique des Matériaux (GPM), Université et INSA de Rouen, UMR 6634, CNRS, Av. de l' Université, BP 12, 76801 Saint Etienne du Rouvray (France); Xu, Tao; Grandidier, Bruno; Stiévenard, Didier [Institut d' Electronique et de Microélectronique et de Nanotechnologies (IEMN), UMR 8520, CNRS, Département ISEN, 41 bd Vauban, 59046 Lille Cedex (France)

    2015-09-14

    By correlating atom probe tomography with other conventional microscope techniques (scanning electron microscope, scanning transmission electron microscope, and scanning tunneling microscopy), the distribution and composition of Au clusters in individual vapor-liquid-solid grown Si nanowires is investigated. Taking advantage of the characteristics of atom probe tomography, we have developed a sample preparation method by inclining the sample at certain angle to characterize the nanowire sidewall without using focused ion beam. With three-dimensional atomic scale reconstruction, we provide direct evidence of Au clusters tending to remain on the nanowire sidewall rather than being incorporated into the Si nanowires. Based on the composition measurement of Au clusters (28% ± 1%), we have demonstrated the supersaturation of Si atoms in Au clusters, which supports the hypothesis that Au clusters are formed simultaneously during nanowire growth rather than during the cooling process.

  5. Atomic characterization of Au clusters in vapor-liquid-solid grown silicon nanowires

    International Nuclear Information System (INIS)

    By correlating atom probe tomography with other conventional microscope techniques (scanning electron microscope, scanning transmission electron microscope, and scanning tunneling microscopy), the distribution and composition of Au clusters in individual vapor-liquid-solid grown Si nanowires is investigated. Taking advantage of the characteristics of atom probe tomography, we have developed a sample preparation method by inclining the sample at certain angle to characterize the nanowire sidewall without using focused ion beam. With three-dimensional atomic scale reconstruction, we provide direct evidence of Au clusters tending to remain on the nanowire sidewall rather than being incorporated into the Si nanowires. Based on the composition measurement of Au clusters (28% ± 1%), we have demonstrated the supersaturation of Si atoms in Au clusters, which supports the hypothesis that Au clusters are formed simultaneously during nanowire growth rather than during the cooling process

  6. Enhanced synthesis of Sn nanowires with aid of Se atom via physical vapor transport

    Science.gov (United States)

    Cai, Huacheng; Wang, Wendong; Liu, Peiwen; Wang, Guangming; Liu, Ankang; He, Zhe; Cheng, Zhaofang; Zhang, Shengli; Xia, Minggang

    2015-06-01

    We demonstrate tin (Sn) nanowires growth enhanced by Selenium (Se) atoms via physical vapor transport (PVT) method. The Raman spectroscopy, X-ray diffraction, scanning electron microscopy and high-resolution transmission electron microscopy show that Sn nanowires are synthesized with a large quantity, good quality and high purity of Sn. The growth of Sn nanowires is attributed to Solid-Vapor-Liquid mechanism. The effects of gold nanoparticles catalyst, Si substrate, and Se atoms on Sn nanowires growth are discussed in detail. We find that Se atom plays a key role in the growth of Sn nanowires. The gaseous Sn atoms are absorbed by the eutectic alloy droplets of Se-Au at first. Then Sn atoms precipitate at the liquid-solid phase interface due to a supersaturated solution and form a one-dimensional nanostructure. In all, this PVT method could provide a simple and quick way to synthesize monocrystalline Sn nanowires with an advantage in both quality and quantity. The optical transmittance of Sn nanowires thin film with 2 μm2 density approaches 85-90% in visible wavelength. Therefore, the Sn nanowires thin film can be applied to transparent electrode along with their metallic property.

  7. Magnetic coupling of laser-cooled atoms to a micro-resonator

    Science.gov (United States)

    Geraci, Andrew; Wang, Ying-Ju; Eardley, Matthew; Moreland, John; Kitching, John

    2009-05-01

    The direct coupling of the spin-degrees of freedom of an atomic vapor to the vibrational motion of a magnetic cantilever tip has recently been demonstrated [1], and prospects for coupling a BEC on an atom-chip to a nano- mechanical resonator have been recently discussed [2]. Possible applications include chip-scale atomic devices, in which localized interactions with magnetic cantilever tips selectively influence or probe atomic spins. As a next step towards the realization of a strongly coupled ultra-cold atom- resonator system, we have constructed an apparatus to study the direct coupling between the spins of trapped laser-cooled Rb atoms and a magnetic tip on a micro-cantilever. The atoms will be loaded into a magnetic trap formed by the cantilever tip and external magnetic fields. The cantilever will be driven capacitively at its resonance frequency, resulting in a coherent precession of the trapped atomic spins with a matching Larmor frequency. Prospects for measuring the back-action of the ensemble of atomic spins on a cantilever beam will also be discussed. [1] Y.-J. Wang,M. Eardley, S. Knappe, J. Moreland, L. Hollberg, and J. Kitching, PRL 97, 227602 (2006). [2] P. Treutlein,D. Hunger, S. Camerer, T. W. Hansch, and J. Reichel, PRL 99, 140403 (2007).

  8. Beam quality of a non-ideal atom laser

    OpenAIRE

    Riou, Jean-Félix; Guerin, William; Le Coq, Yann; Fauquembergue, Marie; Bouyer, Philippe; Josse, Vincent; Aspect, Alain

    2006-01-01

    International audience We study the propagation of a non-interacting atom laser distorted by the strong lensing effect of the Bose-Einstein Condensate (BEC) from which it is outcoupled. We observe a transverse structure containing caustics that vary with the density within the residing BEC. Using WKB approximation, Fresnel-Kirchhoff integral formalism and ABCD matrices, we are able to describe analytically the atom laser propagation. This allows us to characterize the quality of the non-id...

  9. Theoretical tools for atom-laser-beam propagation

    OpenAIRE

    Riou, Jean-Félix; Le Coq, Yann; Impens, François; Guerin, William; Bordé, Christian,; Aspect, Alain; Bouyer, Philippe

    2008-01-01

    We present a theoretical model for the propagation of non self-interacting atom laser beams. We start from a general propagation integral equation, and we use the same approximations as in photon optics to derive tools to calculate the atom laser beam propagation. We discuss the approximations that allow to reduce the general equation whether to a Fresnel-Kirchhoff integral calculated by using the stationary phase method, or to the eikonal. Within the paraxial approximation, we also introduce...

  10. Laser vaporization of cirrus-like ice particles with secondary ice multiplication.

    Science.gov (United States)

    Matthews, Mary; Pomel, François; Wender, Christiane; Kiselev, Alexei; Duft, Denis; Kasparian, Jérôme; Wolf, Jean-Pierre; Leisner, Thomas

    2016-05-01

    We investigate the interaction of ultrashort laser filaments with individual 90-μm ice particles, representative of cirrus particles. The ice particles fragment under laser illumination. By monitoring the evolution of the corresponding ice/vapor system at up to 140,000 frames per second over 30 ms, we conclude that a shockwave vaporization supersaturates the neighboring region relative to ice, allowing the nucleation and growth of new ice particles, supported by laser-induced plasma photochemistry. This process constitutes the first direct observation of filament-induced secondary ice multiplication, a process that strongly modifies the particle size distribution and, thus, the albedo of typical cirrus clouds. PMID:27386537

  11. Chemical oxygen-iodine laser with atomic iodine generated via fluorine atoms

    Czech Academy of Sciences Publication Activity Database

    Špalek, Otomar; Jirásek, Vít; Čenský, Miroslav; Kodymová, Jarmila; Picková, Irena; Jakubec, Ivo

    Bellingham: SPIE, 2007 - (Panchenko, V.; Golubev, V.; Ionin, A.; Chumakov, A.), s. 18-27. (Proceedings of SPIE. 6735). ISBN 978-0-8194-6893-2. ISSN 0277-786X. [International conference on lasers, applications, and technologies 2007: high-power lasers and applications. Minsk (BY), 28.05.2007-01.06.2007] R&D Projects: GA ČR GA202/05/0359 Institutional research plan: CEZ:AV0Z10100523; CEZ:AV0Z40320502 Keywords : atomic iodine * atomic fluorine * chemical oxygen-iodine laser * COIL Subject RIV: BH - Optics, Masers, Lasers

  12. Enhanced light-vapor interactions and all optical switching in a chip scale micro-ring resonator coupled with atomic vapor

    CERN Document Server

    Stern, Liron; Mazurski, Noa; Levy, Uriel

    2016-01-01

    The coupling of atomic and photonic resonances serves as an important tool for enhancing light-matter interactions and enables the observation of multitude of fascinating and fundamental phenomena. Here, by exploiting the platform of atomic-cladding wave guides, we experimentally demonstrate the resonant coupling of rubidium vapor and an atomic cladding micro ring resonator. Specifically, we observed cavity-atom coupling in the form of Fano resonances having a distinct dependency on the relative frequency detuning between the photonic and the atomic resonances. Moreover, we were able to significantly enhance the efficiency of all optical switching in the V-type pump-probe scheme. The coupled system of micro-ring resonator and atomic vapor is a promising building block for a variety of light vapor experiments, as it offers a very small footprint, high degree of integration and extremely strong confinement of light and vapor. As such it may be used for important applications, such as all optical switching, disp...

  13. Space Debris-de-Orbiting by Vaporization Impulse using Short Pulse Laser

    International Nuclear Information System (INIS)

    Space debris constitutes a significant hazard to low earth orbit satellites and particularly to manned spacecraft. A quite small velocity decrease from vaporization impulses is enough to lower the perigee of the debris sufficiently for atmospheric drag to de-orbit the debris. A short pulse (picosecond) laser version of the Orion concept can accomplish this task in several years of operation. The ''Mercury'' short pulse Yb:S-FAP laser being developed at LLNL for laser fusion is appropriate for this task

  14. Efficiency of photodesorption of Rb atoms collected on polymer organic film in vapor-cell

    CERN Document Server

    Atutov, Sergey N; Chubakov, Pavel A; Plekhanov, Alexander I

    2010-01-01

    The efficiency of photodesorption of Rb atoms previously collected on polymer organic film has been studied in detail. This study was carried out in a glass cell of which the inner surface was covered with (poly)dimethylsiloxane (PDMS) film and illuminated by a photographic flash lamp. The desorption dynamic of the Rb atoms density in the cell caused by the illumination was studied using an Rb resonance lamp as a source of probing light. It was determined that about 25 percent of the total Rb atoms embedded on the cell walls can be desorbed by single flash from the lamp and almost 50 percent are desorbed by a sequence of several light pulses. Our result might help to construct an efficient light-driven source of atoms for a new type magneto optical trap for atoms in extremely low vapor density or very weak atomic flux of such artificial alkaline atoms as Francium. We believe that the collection and photodesorption of particles could be used for the development of sensors for the trace detection of various ele...

  15. Cavity atom optics and the `free atom laser'

    OpenAIRE

    Heurich, J.; Moore, M. G.; Meystre, P.

    1999-01-01

    The trap environment in which Bose-Einstein condensates are generated and/or stored strongly influences the way they interact with light. The situation is analogous to cavity QED in quantum optics, except that in the present case, one tailors the matter-wave mode density rather than the density of modes of the optical field. Just as in QED, for short times, the atoms do not sense the trap and propagate as in free space. After times long enough that recoiling atoms can probe the trap environme...

  16. Laser-excitation technique for the measurement of absolute transition probabilities of weak atomic lines

    Science.gov (United States)

    Kwong, H. S.; Smith, P. L.; Parkinson, W. H.

    1982-01-01

    A new technique is presented for the measurement of transition probabilities for weak allowed, intersystem, and forbidden lines. The method exploits the fact that oscillator strength is proportional to the number of stimulated absorptions and emissions produced by a narrow-band laser pulse of known energy which is in resonance with an atomic transition. The method is tested for a particular transition of Mg I with a known oscillator strength value and of appropriate magnitude. The number densities are measured using a Mach-Zehnder interferometer and the hook method for the lower level population and by measuring an absorption-equivalent width for the other. The apparatus consisted of a high-power tunable laser and a magnesium oven to produce excited Mg vapor, and a laser-plasma background continuum. The results are in good agreement with theoretical and other experimental data.

  17. Erbium:YAG-laser induced vapor bubbles as a function of the quartz fiber tip geometry

    Science.gov (United States)

    Mrochen, Michael; Riedel, Peter; Donitzky, Christof; Seiler, Theo

    2001-07-01

    Background. The use of modern erbium: yttrium-aluminum- garnet (YAG) laser systems in ophthalmic microsurgery requires a precise knowledge of the size and dynamics of the laser induced vapor bubbles. The aim of this work was to clarify the possibilities of controlling the vapor bubble shape and size by using an optimized fiber tip geometry for various ophthalmic applications with the erbium:YAG laser. Methods. The mid-infrared radiation of free-running erbium:YAG laser was coupled optically into means of different low OH- quartz fiber tips to investigate the vapor bubble formation in water by high-speed photography. The core diameter of four fiber tips ranged from 200 up to 940 micrometers . Fourteen fiber tips were polished at an angle graduated from 10 degree(s) to 70 degree(s) over the full core diameter (seven fiber tips) and over the half core diameter (seven fiber tips). Three fiber tips were produced to have a curvature at the distal end with curvature radii of 160, 230, and 420 micrometers . Results. The shape as well as the size of erbium:YAG laser induced vapor bubbles can be controlled systematically by using adequate fiber tip geometries. In detail, the used different angles and curvatures demonstrate that the propagation direction of the vapor bubbles can be estimated by optical modeling considering Snell's law and the Fresnel laws at a quartz-air boundary. Beside this, the size of a vapor bubble can be predetermined by choosing ideal fiber tip geometries to reduce or increase the radiant exposure at the distal end of the quartz fiber tip. Conclusions. The good possibility of controlling the shape and size of vapor bubbles offers a wider range of new applications, especially in ophthalmic microsurgery such as erbium YAG laser vitrectomy.

  18. Laser stripping of hydrogen atoms by direct ionization

    International Nuclear Information System (INIS)

    Direct ionization of hydrogen atoms by laser irradiation is investigated as a potential new scheme to generate proton beams without stripping foils. The time-dependent Schroedinger equation describing the atom-radiation interaction is numerically solved obtaining accurate ionization cross-sections for a broad range of laser wavelengths, durations and energies. Parameters are identified where the Doppler frequency up-shift of radiation colliding with relativistic particles can lead to efficient ionization over large volumes and broad bandwidths using currently available lasers

  19. Laserlike and atomlike regimes in a one-atom laser

    OpenAIRE

    Boozer, A. D.

    2008-01-01

    We consider a three-level model of a one-atom laser, and show that there are two limiting regimes of parameter space, one in which the system behaves like a conventional laser and one in which the system exhibits novel quantum properties. We show that in the first limiting regime, the model can be approximated by semiclassical laser theory, and in the second limiting regime the model can be approximated as an effective two-level atom. We also perform numerical simulations that confirm the lim...

  20. Chemical oxygen-iodine laser with atomic iodine generated via fluorine atoms

    Czech Academy of Sciences Publication Activity Database

    Jirásek, Vít; Čenský, Miroslav; Špalek, Otomar; Kodymová, Jarmila; Picková, Irena; Jakubec, Ivo

    2008-01-01

    Roč. 345, č. 1 (2008), 14-22. ISSN 0301-0104 R&D Projects: GA ČR GA202/05/0359 Institutional research plan: CEZ:AV0Z10100523; CEZ:AV0Z40320502 Keywords : atomic iodine * atomic fluorine * chemical oxygen–iodine laser * COIL Subject RIV: BH - Optics, Masers, Lasers Impact factor: 1.961, year: 2008

  1. Laser cooling atoms to indistinguishability: Atomic Hong-Ou-Mandel interference and entanglement through spin exchange

    Science.gov (United States)

    Kaufman, Adam

    2016-05-01

    Motional control of neutral atoms has a rich history and increasingly interest has turned to single-atom control. In my thesis work, we created a platform to individually prepare single bosonic atoms in highly pure quantum states, by developing methods to laser cool single atoms to the vibrational ground state of optical tweezer traps. Applying this toolset, we observe the atomic Hong-Ou-Mandel effect when we arrange for atom tunneling to play the role of a balanced beam splitter between two optical tweezers. In another experiment, we utilize spin exchange to create entanglement, which we then verify after spatially separating the atoms to observe their non-local correlations. Merging these results with our recent demonstration of deterministic loading of atomic arrays, our results establish the concept of quantum gas assembly, which could be applied to a variety of systems ranging from the production of single dipolar molecules to the assembly of low-entropy arrays of atoms.

  2. Probing a Bose-Einstein Condensate with an Atom Laser

    OpenAIRE

    Döring, D.; Robins, N. P.; Figl, C.; Close, J. D.

    2008-01-01

    A pulsed atom laser derived from a Bose-Einstein condensate is used to probe a second target condensate. The target condensate scatters the incident atom laser pulse. From the spatial distribution of scattered atoms, one can infer important properties of the target condensate and its interaction with the probe pulse. As an example, we measure the s-wave scattering length that, in low energy collisions, describes the interaction between the |F=1,m_F=-1> and |F=2,m_F=0> hyperfine ground states ...

  3. Method for laser spectroscopy of metastable pionic helium atoms

    International Nuclear Information System (INIS)

    The PiHe collaboration is currently attempting to carry out laser spectroscopy of metastable pionic helium atoms using the high-intensity π− beam of the ring cyclotron facility of the Paul Scherrer Institute. These atoms are heretofore hypothetical three-body Coulomb systems each composed of a helium nucleus, a π− occupying a Rydberg state, and an electron occupying the 1s ground state. We briefly review the proposed method by which we intend to detect the laser spectroscopic signal. This complements our experiments on metastable antiprotonic helium atoms at CERN

  4. Vapor generation and atom traps: Atomic absorption spectrometry at the ng/L level

    International Nuclear Information System (INIS)

    Atom-trapping atomic absorption spectrometry is a technique that allows detection at the ng/L level for several analytes such as As, Se, Sb, Pb, Bi, Cd, In, Tl, Te, Sn and Hg. The principle involves generation of volatile species, usually hydrides, trapping these species on the surface of an atom trap held at an optimized temperature and, finally, revolatilizing the analyte species by rapid heating of the trap and transporting them in a carrier gas to a heated quartz tube, as commonly used with hydride generation AAS systems. A transient signal having, in most cases, a full width at half maximum of less than 1 s is obtained. The atom trap may be a quartz surface or a W-coil; the former is heated externally and the latter is heated resistively. Both collection and revolatilization temperatures are optimized. In some cases, the W-coil itself is used as an electrothermal atomizer and a heated quartz tube is then not needed. The evolution of these traps starts with the well-known Watling's slotted quartz tube (SQT), continues with atom trapping SQT and finally reaches the present traps mentioned above. The analytical figures of merit for these traps need to be standardized. Naturally, enhancement is on characteristic concentration, C0, where the change in characteristic mass, m0, can be related to trapping efficiency. Novel terms are suggested for E, enhancement factor; such as Emax, maximum enhancement factor; Et, enhancement for 1.0 minute sampling and Ev, enhancement for 1.0 mL of sample. These figures will allow easy comparison of results from different laboratories as well as different analytes and/or traps

  5. Vapor generation and atom traps: Atomic absorption spectrometry at the ng/L level

    Energy Technology Data Exchange (ETDEWEB)

    Ataman, O. Yavuz [Department of Chemistry, Middle East Technical University, 06531 Ankara (Turkey)], E-mail: ataman@metu.edu.tr

    2008-08-15

    Atom-trapping atomic absorption spectrometry is a technique that allows detection at the ng/L level for several analytes such as As, Se, Sb, Pb, Bi, Cd, In, Tl, Te, Sn and Hg. The principle involves generation of volatile species, usually hydrides, trapping these species on the surface of an atom trap held at an optimized temperature and, finally, revolatilizing the analyte species by rapid heating of the trap and transporting them in a carrier gas to a heated quartz tube, as commonly used with hydride generation AAS systems. A transient signal having, in most cases, a full width at half maximum of less than 1 s is obtained. The atom trap may be a quartz surface or a W-coil; the former is heated externally and the latter is heated resistively. Both collection and revolatilization temperatures are optimized. In some cases, the W-coil itself is used as an electrothermal atomizer and a heated quartz tube is then not needed. The evolution of these traps starts with the well-known Watling's slotted quartz tube (SQT), continues with atom trapping SQT and finally reaches the present traps mentioned above. The analytical figures of merit for these traps need to be standardized. Naturally, enhancement is on characteristic concentration, C{sub 0}, where the change in characteristic mass, m{sub 0}, can be related to trapping efficiency. Novel terms are suggested for E, enhancement factor; such as E{sub max}, maximum enhancement factor; E{sub t}, enhancement for 1.0 minute sampling and E{sub v}, enhancement for 1.0 mL of sample. These figures will allow easy comparison of results from different laboratories as well as different analytes and/or traps.

  6. Vapor generation and atom traps: Atomic absorption spectrometry at the ng/L level

    Science.gov (United States)

    Ataman, O. Yavuz

    2008-08-01

    Atom-trapping atomic absorption spectrometry is a technique that allows detection at the ng/L level for several analytes such as As, Se, Sb, Pb, Bi, Cd, In, Tl, Te, Sn and Hg. The principle involves generation of volatile species, usually hydrides, trapping these species on the surface of an atom trap held at an optimized temperature and, finally, revolatilizing the analyte species by rapid heating of the trap and transporting them in a carrier gas to a heated quartz tube, as commonly used with hydride generation AAS systems. A transient signal having, in most cases, a full width at half maximum of less than 1 s is obtained. The atom trap may be a quartz surface or a W-coil; the former is heated externally and the latter is heated resistively. Both collection and revolatilization temperatures are optimized. In some cases, the W-coil itself is used as an electrothermal atomizer and a heated quartz tube is then not needed. The evolution of these traps starts with the well-known Watling's slotted quartz tube (SQT), continues with atom trapping SQT and finally reaches the present traps mentioned above. The analytical figures of merit for these traps need to be standardized. Naturally, enhancement is on characteristic concentration, C0, where the change in characteristic mass, m0, can be related to trapping efficiency. Novel terms are suggested for E, enhancement factor; such as Emax, maximum enhancement factor; Et, enhancement for 1.0 minute sampling and Ev, enhancement for 1.0 mL of sample. These figures will allow easy comparison of results from different laboratories as well as different analytes and/or traps.

  7. Solar-simulator-pumped atomic iodine laser kinetics

    Science.gov (United States)

    Wilson, H. W.; Raju, S.; Shiu, Y. J.

    1983-01-01

    The literature contains broad ranges of disagreement in kinetic data for the atomic iodine laser. A kinetic model of a solar-simulator-pumped iodine laser is used to select those kinetic data consistent with recent laser experiments at the Langley Research Center. Analysis of the solar-simulator-pumped laser experiments resulted in the following estimates of rate coefficients: for alkyl radical (n-C3F7) and atomic iodine (I) recombination, 4.3 x 10 to the 11th power (1.9) + or - cu cm/s; for n-C3F7I stabilized atomic iodine recombination (I + I) 3.7 x 10 to the -32nd power (2.3) + or -1 cm to the 6th power/s; and for molecular iodine (I2) quenching, 3.1 x 10 to the -11th power (1.6) + or - 1 cu cm/s. These rates are consistent with the recent measurements.

  8. Optical measurements of strong microwave fields with Rydberg atoms in a vapor cell

    CERN Document Server

    Anderson, David A; Gordon, Joshua A; Butler, Miranda L; Holloway, Christopher L; Raithel, Georg

    2016-01-01

    We present a spectral analysis of Rydberg atoms in strong microwave fields using electromagnetically induced transparency (EIT) as an all-optical readout. The measured spectroscopic response enables optical, atom-based electric field measurements of high-power microwaves. In our experiments, microwaves are irradiated into a room-temperature rubidium vapor cell. The microwaves are tuned near the two-photon 65D-66D Rydberg transition and reach an electric field strength of 230V/m, about 20% of the microwave ionization threshold of these atoms. A Floquet treatment is used to model the Rydberg level energies and their excitation rates. We arrive at an empirical model for the field-strength distribution inside the spectroscopic cell that yields excellent overall agreement between the measured and calculated Rydberg EIT-Floquet spectra. Using spectral features in the Floquet maps we achieve an absolute strong-field measurement precision of 6%.

  9. Optical Measurements of Strong Microwave Fields with Rydberg Atoms in a Vapor Cell

    Science.gov (United States)

    Anderson, D. A.; Miller, S. A.; Raithel, G.; Gordon, J. A.; Butler, M. L.; Holloway, C. L.

    2016-03-01

    We present a spectral analysis of Rydberg atoms in strong microwave fields using electromagnetically induced transparency (EIT) as an all-optical readout. The measured spectroscopic response enables optical, atom-based electric-field measurements of high-power microwaves. In our experiments, microwaves are irradiated into a room-temperature rubidium vapor cell. The microwaves are tuned near the two-photon 65 D -66 D Rydberg transition and reach an electric-field strength of 230 V /m , about 20% of the microwave-ionization threshold of these atoms. A Floquet treatment is used to model the Rydberg-level energies and their excitation rates. We arrive at an empirical model for the field-strength distribution inside the spectroscopic cell that yields excellent overall agreement between the measured and calculated Rydberg EIT-Floquet spectra. Using spectral features in the Floquet maps, we achieve an absolute strong-field measurement precision of 6%.

  10. Imaging Microwave and DC Magnetic Fields in a Vapor-Cell Rb Atomic Clock

    CERN Document Server

    Affolderbach, Christoph; Bandi, Thejesh; Horsley, Andrew; Treutlein, Philipp; Mileti, Gaetano

    2015-01-01

    We report on the experimental measurement of the DC and microwave magnetic field distributions inside a recently-developed compact magnetron-type microwave cavity, mounted inside the physics package of a high-performance vapor-cell atomic frequency standard. Images of the microwave field distribution with sub-100 $\\mu$m lateral spatial resolution are obtained by pulsed optical-microwave Rabi measurements, using the Rb atoms inside the cell as field probes and detecting with a CCD camera. Asymmetries observed in the microwave field images can be attributed to the precise practical realization of the cavity and the Rb vapor cell. Similar spatially-resolved images of the DC magnetic field distribution are obtained by Ramsey-type measurements. The T2 relaxation time in the Rb vapor cell is found to be position dependent, and correlates with the gradient of the DC magnetic field. The presented method is highly useful for experimental in-situ characterization of DC magnetic fields and resonant microwave structures,...

  11. Determination of cadmium in water samples by fast pyrolysis-chemical vapor generation atomic fluorescence spectrometry

    Science.gov (United States)

    Zhang, Jingya; Fang, Jinliang; Duan, Xuchuan

    2016-08-01

    A pyrolysis-vapor generation procedure to determine cadmium by atomic fluorescence spectrometry has been established. Under fast pyrolysis, cadmium ion can be reduced to volatile cadmium species by sodium formate. The presence of thiourea enhanced the efficiency of cadmium vapor generation and eliminated the interference of copper. The possible mechanism of vapor generation of cadmium was discussed. The optimization of the parameters for pyrolysis-chemical vapor generation, including pyrolysis temperature, amount of sodium formate, concentration of hydrochloric acid, and carrier argon flow rate were carried out. Under the optimized conditions, the absolute and concentration detection limits were 0.38 ng and 2.2 ng ml- 1, respectively, assuming that 0.17 ml of sample was injected. The generation efficiency of was 28-37%. The method was successfully applied to determine trace amounts of cadmium in two certified reference materials of Environmental Water (GSB07-1185-2000 and GSBZ 50009-88). The results were in good agreement with the certified reference values.

  12. Laser Assisted Free-Free Transition in Electron - Atom Collision

    Science.gov (United States)

    Sinha, C.; Bhatia, A. K.

    2011-01-01

    Free-free transition is studied for electron-Hydrogen atom system in ground state at very low incident energies in presence of an external homogeneous, monochromatic and linearly polarized laser field. The incident electron is considered to be dressed by the laser in a non perturbative manner by choosing the Volkov solutions in both the channels. The space part of the scattering wave function for the electron is solved numerically by taking into account the effect of electron exchange, short range as well as of the long range interactions. Laser assisted differential as well as elastic total cross sections are calculated for single photon absorption/emission in the soft photon limit, the laser intensity being much less than the atomic field intensity. A strong suppression is noted in the laser assisted cross sections as compared to the field free situations. Significant difference is noted in the singlet and the triplet cross sections.

  13. Probing temperature during laser spot welding from vapor composition and modeling

    Science.gov (United States)

    He, X.; DebRoy, T.; fürschbach, P. W.

    2003-11-01

    Measurement of weld pool temperature during laser spot welding is a difficult task because of the short pulse duration, often lasting only a few milliseconds, highly transient nature of the process, and the presence of a metal vapor plume near the weld pool. This article describes recent research to estimate weld pool temperatures experimentally and theoretically. Composition of the metal vapor from the weld pool was determined by condensing a portion of the vapor on the inner surface of an open ended quartz tube which was mounted perpendicular to the sample surface and coaxial with the laser beam. It was found that iron, chromium, and manganese were the main metallic species in the vapor phase. The concentrations of Fe and Cr in the vapor increased slightly while the concentration of Mn in the vapor decreased somewhat with the increase in power density. The vapor composition was used to determine an effective temperature of the weld pool. A transient, three-dimensional numerical heat transfer and fluid flow model based on the solution of the equations of conservation of mass, momentum and energy was used to calculate the temperature and velocity fields in the weld pool as a function of time. The experimentally determined geometry of the spot welds agreed well with that determined from the computed temperature field. The effective temperature determined from the vapor composition was found to be close to the numerically computed peak temperature at the weld pool surface. Because of the short process duration and other serious problems in the direct measurement of temperature during laser spot welding, estimating approximate values of peak temperature from metal vapor composition is particularly valuable.

  14. Probing temperature during laser spot welding from vapor composition and modeling

    International Nuclear Information System (INIS)

    Measurement of weld pool temperature during laser spot welding is a difficult task because of the short pulse duration, often lasting only a few milliseconds, highly transient nature of the process, and the presence of a metal vapor plume near the weld pool. This article describes recent research to estimate weld pool temperatures experimentally and theoretically. Composition of the metal vapor from the weld pool was determined by condensing a portion of the vapor on the inner surface of an open ended quartz tube which was mounted perpendicular to the sample surface and coaxial with the laser beam. It was found that iron, chromium, and manganese were the main metallic species in the vapor phase. The concentrations of Fe and Cr in the vapor increased slightly while the concentration of Mn in the vapor decreased somewhat with the increase in power density. The vapor composition was used to determine an effective temperature of the weld pool. A transient, three-dimensional numerical heat transfer and fluid flow model based on the solution of the equations of conservation of mass, momentum and energy was used to calculate the temperature and velocity fields in the weld pool as a function of time. The experimentally determined geometry of the spot welds agreed well with that determined from the computed temperature field. The effective temperature determined from the vapor composition was found to be close to the numerically computed peak temperature at the weld pool surface. Because of the short process duration and other serious problems in the direct measurement of temperature during laser spot welding, estimating approximate values of peak temperature from metal vapor composition is particularly valuable

  15. Atomic physics experiments combining synchrotron radiation and lasers: present capabilities and future possibilities

    International Nuclear Information System (INIS)

    This (occasionally speculative) paper considers the range of hybrid experiments in atomic physics that are now or may soon be possible with combined use of two rather different photon sources, monochromatized synchrotron radiation (SR) in the vacuum ultraviolet (VUV) below about 300 eV and lasers below about 5-10 eV. A wide range of experiments will employ one or more continuous lasers to create an appreciable stationary fraction of valence-excited target atoms in a beam and will draw heavily on the techniques previously developed to create aligned or oriented targets for electron scattering experiments. The very low duty factor of most pulsed lasers mitigates against their use with SR, but it should be possible to develop specialized, mode-locked, pulsed dye lasers whose pulse train is synchronized to that of the SR source. The development of free-electron lasers at SR facilities will provide an ideal tunable laser source in the same laboratories, certainly in the infrared and perhaps into the UV. SR and photoelectron spectroscopy can be used to probe photo-excitation and ionization of electrons in inner or outer shells, either directly or via doubly-excited resonances. Triply-excited states may also be open to study. Analogous experiments with electronically or vibronically excited molecules will be challenging. In laser-excited alkali and alkaline-earth vapors, collisional interactions among the excited atoms can produce a weakly ionized plasma emitting hot electrons that can confuse SR photoelectron spectra, especially near ionization thresholds. 33 references, 2 figures, 3 tables

  16. Feshbach-resonance-induced atomic filamentation and quantum pair correlation in atom-laser-beam propagation

    OpenAIRE

    Zhang, Weiping; Search, Chris P.; Pu, Han; Meystre, Pierre; Wright, Ewan M.

    2002-01-01

    We study the propagation of an atom laser beam through a spatial region with a magnetic field tuned to a Feshbach resonance. Tuning the magnetic field below the resonance produces an effective focusing Kerr medium that causes a modulational instability of the atomic beam. Under appropriate circumstances, this results in beam breakup and filamentation seeded by quasi-particle fluctuations, and in the generation of correlated atomic pairs.

  17. The Synthesized of Carbon Nano tubes from Palm Oil by Topas Atomizer Chemical Vapor Deposition Method

    International Nuclear Information System (INIS)

    This paper focused on preparation of Carbon Nano tubes (CNTs) based on palm oil as a natural resource precursor. The Topas Atomizer was utilized to vapor up the carbon gas into the reaction chamber of Chemical Vapor Deposition (CVD) to yield the CNTs in powder form at the inner wall of the Quartz tube. The purpose of this work was to investigate the effects of deposition temperature from 650 - 850 degree Celsius. The samples characteristics were analyzed by Raman spectroscopy. The results revealed that the increasing of the deposition temperature, the ID/IG ratio decreased from 650 - 850 degree Celsius. The results of Field Emission Scanning Electron Microscopy (FESEM) are also presented. (author)

  18. Chemical vapor deposition of atomically thin materials for membrane dialysis applications

    Science.gov (United States)

    Kidambi, Piran; Mok, Alexander; Jang, Doojoon; Boutilier, Michael; Wang, Luda; Karnik, Rohit; Microfluidics; Nanofluidics Research Lab Team

    2015-11-01

    Atomically thin 2D materials like graphene and h-BN represent a new class of membranes materials. They offer the possibility of minimum theoretical membrane transport resistance along with the opportunity to tune pore sizes at the nanometer scale. Chemical vapor deposition has emerged as the preferable route towards scalable, cost effective synthesis of 2D materials. Here we show selective molecular transport through sub-nanometer diameter pores in graphene grown via chemical vapor deposition processes. A combination of pressure driven and diffusive transport measurements shows evidence for size selective transport behavior which can be used for separation by dialysis for applications such as desalting of biomolecular or chemical solutions. Principal Investigator

  19. Laser-induced fluorescence studies of polycyclic aromatic hydrocarbons (PAH) vapors at high temperatures.

    Science.gov (United States)

    Chi, Z; Cullum, B M; Stokes, D L; Mobley, J; Miller, G H; Hajaligol, M R; Vo-Dinh, T

    2001-06-01

    In this work, we present the fluorescence spectra of anthracene and pyrene vapors at different elevated temperatures (from 150 to 650 degrees C) excited with the 337 nm line of a nitrogen laser. We describe the high temperature effects on the resulting spectral properties including spectral intensity, spectral bandwidth and spectral shift. We found that the PAH fluorescence spectral bandwidths become very broad as the temperature increases. The broadening is mainly due to thermal vibrational sequence congestion. We also have found that the fluorescence intensity of pyrene vapor increases with increasing temperature, which results from the increase of the pyrene vapor absorption cross section at 337 nm. PMID:11446693

  20. Simulation of Chromium Atom Deposition Pattern in a Gaussain Laser Standing Wave with Different Laser Power

    Institute of Scientific and Technical Information of China (English)

    ZHANG Wen-Tao; ZHU Bao-Hua

    2009-01-01

    One-dimensional deposition of a neutral chromium atomic beam focused by a near-resonant Gaussian standing-laser field is discussed by using a fourth-order Runge-Kutta type algorithm. The deposition pattern of neutral chromium atoms in a laser standing wave with different laser power is discussed and the simulation result shows that the full width at half maximum (FWHM) of a nanometer stripe is 115nm and the contrast is 2.5:1 with laser power 3.93mW; the FWHM is 0.Snm and the contrast is 27:1 with laser power 16mW, the optimal laser power; but with laser power increasing to 50mW, the nanometer structure forms multi-crests and the quality worsens quickly with increasing laser power.

  1. Proposed search for an electric-dipole moment using laser-cooled $^{171}$Yb atoms

    CERN Document Server

    Natarajan, V

    2005-01-01

    We propose an experiment to search for a permanent atomic electric-dipole moment (EDM) using laser-cooled $^{171}$Yb atoms launched in an atomic fountain. A uniform B field sets the quantization axis, and the Ramsey separated-oscillatory-fields method is used to measure the Zeeman precession frequency of the atoms. Laser beams of appropriate polarization are used for preparation and detection in a given magnetic sublevel. The signature of an EDM is a shift in the Ramsey resonance correlated with application of a large E field. The precision is expected to be at least 20 times better than current limits because the use of a cold atomic beam allows application of E field 10 times larger than in a vapor cell, and the interaction time with the E field is 200 times larger compared to a thermal beam. The leading source of systematic error in beam experiments, the (E x v/c) motional magnetic field, is reduced considerably because of the near-perfect reversal of velocity between up and down trajectories through the E...

  2. Proposed search for an electric-dipole moment using laser-cooled 171Yb atoms

    International Nuclear Information System (INIS)

    The existence of a permanent electric-dipole moment (EDM) in a particle implies that both parity (P) and time-reversal symmetry (T) are violated. We propose an experiment to search for a permanent atomic EDM using laser-cooled 171Yb atoms launched in an atomic fountain. A uniform B field sets the quantization axis, and the Ramsey separated-oscillatory-fields method is used to measure the Zeeman precession frequency of the atoms. Laser beams of appropriate polarization are used for preparation and detection in a given magnetic sub-level. The signature of an EDM is a shift in the Ramsey resonance correlated with application of a large E field. The precision is expected to be at least 20 times better than current limits because the use of a cold atomic beam allows application of E field 10 times larger than in a vapor cell, and the interaction time with the E field is 200 times larger compared to a thermal beam. The leading source of systematic error in beam experiments, the motional magnetic field, is reduced considerably because of the near-perfect reversal of velocity between up and down trajectories through the E-field region. (authors)

  3. Recirculation of Laser Power in an Atomic Fountain

    Science.gov (United States)

    Enzer, Daphna G.; Klipstein, WIlliam M.; Moore, James D.

    2007-01-01

    A new technique for laser-cooling atoms in a cesium atomic fountain frequency standard relies on recirculation of laser light through the atom-collection region of the fountain. The recirculation, accomplished by means of reflections from multiple fixed beam-splitter cubes, is such that each of two laser beams makes three passes. As described below, this recirculation scheme offers several advantages over prior designs, including simplification of the laser system, greater optical power throughput, fewer optical and electrical connections, and simplification of beam power balancing. A typical laser-cooled cesium fountain requires the use of six laser beams arranged as three orthogonal pairs of counter-propagating beams to decelerate the atoms and hold them in a three-dimensional optical trap in vacuum. Typically, these trapping/cooling beams are linearly polarized and are positioned and oriented so that (1) counter-propagating beams in each pair have opposite linear polarizations and (2) three of the six orthogonal beams have the sum of their propagation directions pointing up, while the other three have the sum of their propagation directions pointing down. In a typical prior design, two lasers are used - one to generate the three "up" beams, the other to generate the three "down" beams. For this purpose, the output of each laser is split three ways, then the resulting six beams are delivered to the vacuum system, independently of each other, via optical fibers. The present recirculating design also requires two lasers, but the beams are not split before delivery. Instead, only one "up" beam and one oppositely polarized "down" beam are delivered to the vacuum system, and each of these beams is sent through the collection region three times. The polarization of each beam on each pass through the collection region is set up to yield the same combination of polarization and propagation directions as described above. In comparison with the prior design, the present

  4. Laser pulse propagation in a meter scale rubidium vapor/plasma cell in AWAKE experiment

    Science.gov (United States)

    Joulaei, A.; Moody, J.; Berti, N.; Kasparian, J.; Mirzanejhad, S.; Muggli, P.

    2016-09-01

    We present the results of numerical studies of laser pulse propagating in a 3.5 cm Rb vapor cell in the linear dispersion regime by using a 1D model and a 2D code that has been modified for our special case. The 2D simulation finally aimed at finding laser beam parameters suitable to make the Rb vapor fully ionized to obtain a uniform, 10 m-long, at least 1 mm in radius plasma in the next step for the AWAKE experiment.

  5. Laser pulse propagation in a meter scale rubidium vapor/plasma cell in AWAKE experiment

    CERN Document Server

    Joulaei, Atefeh; Berti, Nicolas; Kasparian, Jerome; Mirzanejhad, Saeed; Muggli, Patric

    2015-01-01

    We present the results of numerical studies of laser pulse propagating in a 3.5 cm Rb vapor cell in the linear dispersion regime by using a 1D model and a 2D code that has been modified for our special case. The 2D simulation finally aimed at finding laser beam parameters suitable to make the Rb vapor fully ionized to obtain a uniform, 10 m-long, at least 1 mm in radius plasma in the next step for the AWAKE experiment.

  6. LASER-INDUCED DECOMPOSITION OF METAL CARBONYLS FOR CHEMICAL VAPOR DEPOSITION OF MICROSTRUCTURES

    OpenAIRE

    Tonneau, D.; Auvert, G.; Pauleau, Y.

    1989-01-01

    Tungsten and nickel carbonyls were used to produce metal microstructures by laser-induced chemical vapor deposition (CVD) on various substrates. The deposition rate of microstructures produced by thermodecomposition of W(CO)6 on Si substrates heated with a cw Ar+ laser beam was relatively low (10 to 30 nm/s) even at high temperatures (above 900°C). Ni microstructures were deposited on quartz substrates irradiated with a CO2 laser beam. Relatively high laser powers were needed to heat the Ni s...

  7. Laser cooling and trapping of atoms

    OpenAIRE

    Townsend Christopher G.

    1995-01-01

    A detailed experimental and theoretical investigation of a magneto-optical trap for caesium atoms is presented. Particular emphasis has been placed on achieving high spatial number densities and low temperatures. Optimizing both of these together enables efficient evaporative cooling from a conservative trap, a procedure which has recently led to the first observations of Bose-Einstein condensation in a dilute atomic vapour. The behaviour of a magneto-optical trap is nomina...

  8. A CPT-based Cs vapor cell atomic clock with a short-term fractional frequency stability of 3 x 10-13 τ-1/2

    Science.gov (United States)

    Abdel Hafiz, Moustafa; Liu, Xiaochi; Guérandel, Stéphane; De Clercq, Emeric; Boudot, Rodolphe

    2016-06-01

    This article reports on the development and short-term fractional frequency stability of a continuous-regime (CW) Cs vapor cell atomic clock based on coherent population trapping (CPT). The push-pull optical pumping technique is used to increase the number of atoms that participate to the clock transition, yielding a typical CPT resonance contrast of 25% for a CPT linewidth of about 450 Hz. The clock short-term fractional frequency stability is measured to be 3 x 10-13 τ-1/2 up to 100 seconds averaging time, in correct agreement with the signal-to-noise ratio limit. The mid-term frequency stability results are currently mainly limited by laser power effects. The detection of high-contrast narrow Raman-Ramsey fringes is demonstrated with this setup by making the atoms interact with a light pulse sequence.

  9. Modulation of the photonic band structure topology of a honeycomb lattice in an atomic vapor

    CERN Document Server

    Zhang, Yiqi; Belić, Milivoj R; Wu, Zhenkun; Zhang, Yanpeng

    2015-01-01

    In an atomic vapor, a honeycomb lattice can be constructed by utilizing the three-beam interference method. In the method, the interference of the three beams splits the dressed energy level periodically, forming a periodic refractive index modulation with the honeycomb profile. The energy band topology of the honeycomb lattice can be modulated by frequency detunings, thereby affecting the appearance (and disappearance) of Dirac points and cones in the momentum space. This effect can be usefully exploited for the generation and manipulation of topological insulators.

  10. Amplified light storage with high fidelity based on electromagnetically induced transparency in rubidium atomic vapor

    Science.gov (United States)

    Zhou, Wei; Wang, Gang; Tang, Guoyu; Xue, Yan

    2016-06-01

    By using slow and stored light based on electromagnetically induced transparency (EIT), we theoretically realize the storage of optical pulses with enhanced efficiency and high fidelity in ensembles of warm atoms in 85Rb vapor cells. The enhancement of storage efficiency is achieved by introducing a pump field beyond three-level configuration to form a N-type scheme, which simultaneously inhibits the undesirable four-wave mixing effect while preserves its fidelity. It is shown that the typical storage efficiency can be improved from 29% to 53% with the application of pump field. Furthermore, we demonstrate that this efficiency decreases with storage time and increases over unity with optical depth.

  11. Direct observation of population transfer between the upper laser levels in a copper vapor laser

    International Nuclear Information System (INIS)

    The copper vapor laser (CVL) produces output at two wavelengths, 511 and 578 nm. These lines do not have common upper or lower levels. It would be extremely desirable to be able to extract the population of both upper levels on one transition only. Whether this is feasible depends critically on the extent to which the population can be transferred between them during a laser pulse. There are several mechanisms which might cause such population transfer: copper-copper, copper-buffer gas, and coper-electron collisions. In normal lasing conditions, calculations indicate that copper-buffer gas collisions should dominate over copper-copper collisions. There are insufficient data to predict whether copper-electron collisions are competitive. The authors have performed a series of experiments in a 10-W CVL (25-mm i.d., 700 mm long) to study the population transfer mechanisms in optimum lasing conditions. They conclude that, although population transfer between the upper levels of a CVL occurs, it does not play an important role in CVL kinetics

  12. Laser-induced atomic adsorption: a mechanism for nanofilm formation

    CERN Document Server

    Martins, Weliton S; Oriá, Marcos; Chevrollier, Martine

    2013-01-01

    We demonstrate and interpret a technique of laser-induced formation of thin metallic films using alkali atoms on the window of a dense-vapour cell. We show that this intriguing photo-stimulated process originates from the adsorption of Cs atoms via the neutralisation of Cs$^+$ ions by substrate electrons. The Cs$^+$ ions are produced via two-photon absorption by excited Cs atoms very close to the surface, which enables the transfer of the laser spatial intensity profile to the film thickness. An initial decrease of the surface work function is required to guarantee Cs$^+$ neutralisation and results in a threshold in the vapour density. This understanding of the film growth mechanism may facilitate the development of new techniques of laser-controlled lithography, starting from thermal vapours.

  13. Rate-equation approach to atomic-laser light statistics

    CERN Document Server

    Chusseau, L; Philippe, F; Chusseau, Laurent; Arnaud, Jacques; Philippe, Fabrice

    2002-01-01

    We consider three- and four-level atomic lasers that are either incoherently (unidirectionally) or coherently (bidirectionally) pumped, the single-mode cavity being resonant with the laser transition. The intra-cavity Fano factor and the photo-current spectral density are evaluated on the basis of rate equations. According to that approach, fluctuations are caused by jumps in active and detecting atoms. The algebra is considerably simpler than the one required by Quantum-Optics treatments. Whenever a comparison can be made, the expressions obtained coincide. The conditions under which the output light exhibits sub-Poissonian statistics are considered in detail. Analytical results, based on linearization, are verified by comparison with Monte Carlo simulations. An essentially exhaustive investigation of sub-Poissonian light generation by three- and four-level atoms lasers has been performed. Only special forms were reported earlier.

  14. Theoretical Femtosecond Physics Atoms and Molecules in Strong Laser Fields

    CERN Document Server

    Grossmann, Frank

    2008-01-01

    Theoretical femtosecond physics is a new field of research. Theoretical investigations of atoms and molecules interacting with pulsed or continuous wave lasers of up to atomic field strengths are leading to an understanding of many challenging experimental discoveries. Laser-matter interaction is treated on a nonperturbative level in the book using approximate and numerical solutions of the time-dependent Schrödinger equation. The light field is treated classically. Physical phenomena, ranging from ionization of atoms to the ionization and dissociation of molecules and the control of chemical reactions are presented and discussed. Theoretical background for experiments with strong and short laser pulses is given. Several exercises are included in the main text. Some detailed calculations are performed in the appendices.

  15. Laser sources for precision spectroscopy on atomic strontium

    OpenAIRE

    Poli, N.; Ferrari, G; Prevedelli, M.; Sorrentino, F.; Drullinger, R. E.; Tino, G. M.

    2006-01-01

    We present a new laser setup designed for high-precision spectroscopy on laser cooled atomic strontium. The system, which is entirely based on semiconductor laser sources, delivers 200 mW at 461 nm for cooling and trapping atomic strontium from a thermal source, 4 mW at 497 nm for optical pumping from the metastable View the MathML source state, 12 mW at 689 nm on linewidth less than 1 kHz for second-stage cooling of the atomic sample down to the recoil limit, 1.2 W at 922 nm for optical trap...

  16. Effect of atomic noise on optical squeezing via polarization self-rotation in a thermal vapor cell

    DEFF Research Database (Denmark)

    Hsu, M.T.L.; Hetet, G.; Peng, A.; Harb, C.C.; Bachor, H.-A.; Johnsson, M.T.; Hope, J.J.; Lam, P.K.; Dantan, Aurelien Romain; Cviklinski, J.; Bramati, A.; Pinard, M.

    2006-01-01

    show results of the characterization of PSR in isotopically enhanced rubidium-87 cells, performed in two independent laboratories. We observed that, contrary to earlier work, the presence of atomic noise in the thermal vapor overwhelms the observation of squeezing. We present a theory that contains...... atomic noise terms and show that a null result in squeezing is consistent with this theory....

  17. Laser vaporization in treatment of superficial endometriosis of the uterine cervix

    Science.gov (United States)

    Wozniak, Jakub; Wilczak, Maciej; Opala, Tomasz; Pisarska-Krawczyk, Magdalena; Cwojdzinski, Marek; Pisarski, Tadeusz

    1996-03-01

    The study shows the treatment of superficial endometriosis of the uterine cervix in 79 patients. After first vaporization 74 patients were cured successfully. In two cases the laser procedure should be repeated and in 3 women the operation should be performed for the third time. All patients are still under control in our department and there is no recurrence observed. Carbon- dioxide laser vaporization under colposcopic control is an efficient method of treatment of superficial endometriosis of the uterine cervix that requires no anaesthesia. The healing process after laser procedures is fast and without complications. The number of recurrences is low. Use of carbon-dioxide laser under colposcopic control because of precise destruction of lesions, fast healing and a low number of recurrences seems to be the method of choice.

  18. A real time Monte Carlo simulation of thin film nucleation in localized-laser chemical vapor deposition

    Science.gov (United States)

    Kotecki, David E.; Herman, Irving P.

    1988-11-01

    A real time Monte Carlo simulation is used to model the nucleation and initial stages of thin film growth during localized-laser chemical vapor deposition (LLCVD). This model includes the effects of laser-substrate heating, heterogeneous pyrolytic decomposition of parent molecules on the laser-heated region of the surface, and adatom migration and desorption dynamics. The amount of material deposited as a function of time is obtained over a surface area of 150×150 Å for various values of the substrate temperature, parent gas pressure, and adsorbate-substrate binding energy. Additional information is obtained about the cluster density, and the role of surface defects and two-atom cluster dynamics on the initial growth rate. The deposition of silicon by heterogeneous pyrolytic decomposition of silane (SiH4) is used as a base case for the simulation. Predictions of the initial thin film morphology and its temporal evolution during static laser heating of micron-dimensional regions of the surface are presented. Simulation results indicate that for a given silane pressure and adsorbate-substrate binding energy, there is a critical temperature Tc such that for laser-induced peak temperatures TpTc, nucleation occurs initially in an annulus region centered with respect to the incident laser irradiation. The inclusion of two-atom cluster dynamics in the simulation is shown to increase the value of Tc and alter the initial morphology for low adsorbate-substrate binding energies. The simulation results are extended to scanning LLCVD to predict the maximum scan speed at which nucleation will occur.

  19. CW fountain of laser-cooled Yb atoms

    CERN Document Server

    Rathod, K D; Natarajan, Vasant

    2013-01-01

    We demonstrate launching of laser-cooled Yb atoms in a continuous atomic fountain. The continuous fountain has significant advantages over the more common pulsed fountain, which was also demonstrated by us recently. The fountain is formed in the following steps---(i) Atoms from a thermal beam are first Zeeman slowed to a small final velocity, (ii) the slowed atoms are captured in a two-dimensional magneto-optic trap (2D-MOT), and (iii) atoms are launched {\\em continuously} in the vertical direction using two sets of moving-molasses beams, inclined at $\\pm 15^\\circ$ to the vertical. The cooling transition used is the strongly-allowed ${^1S}_0 \\rightarrow {^1P}_1$ transition at 399 nm. We capture about $7 \\times 10^6$ atoms in the 2D-MOT, and then launch them with a vertical velocity of 13 m/s at a longitudinal temperature of 125(6) mK.

  20. Frequency-Tunable Microwave Field Detection in an Atomic Vapor Cell

    CERN Document Server

    Horsley, Andrew

    2016-01-01

    We use an atomic vapor cell as a frequency tunable microwave field detector operating at frequencies from GHz to tens of GHz. We detect microwave magnetic fields from 2.3 GHz to 26.4 GHz, and measure the amplitude of the sigma+ component of an 18 GHz microwave field. Our proof-of-principle demonstration represents a four orders of magnitude extension of the frequency tunable range of atomic magnetometers from their previous dc to several MHz range. When integrated with a high resolution microwave imaging system, this will allow for the complete reconstruction of the vector components of a microwave magnetic field and the relative phase between them. Potential applications include near-field characterisation of microwave circuitry and devices, and medical microwave sensing and imaging.

  1. Suppressing decoherence of spin waves in a warm atomic vapor by applying a guiding magnetic field

    International Nuclear Information System (INIS)

    We report an experimental and theoretical investigation to extend lifetimes of light storages by applying guiding magnetic fields in a room-temperature atomic vapor. The storages are based on dynamic electromagnetically induced transparency. Retrieval efficiencies versus storage time are experimentally measured for different strengths of the guiding magnetic fields. The measured results show that the 1/e storage times are ∼6 μs and ∼59 μs for the guiding field B0z = 0 and B0z = 93 mG, respectively. Physical processes causing decoherence in an atomic ensemble have been discussed and analyzed. A theory model which is used to evaluate the decoherence caused by fluctuations of transverse magnetic fields is developed. Based on this evaluation, the fact that storage lifetimes can be increased by applying guiding magnetic fields is well explained. (paper)

  2. Spectral and angular features of the propagation of an intense laser wave through sodium vapor

    International Nuclear Information System (INIS)

    An experimental study of the propagation of intense laser light in a resonant medium (sodium vapor) has revealed a scattering component which is inconsistent with the Raman scattering spectra of a three-level system in an intense laser field. Spectral and angular characteristics of this component have been studied. It is shown that the occurrence of this component can be explained by a model of a resonant four-wave mixing. 6 refs., 2 figs

  3. Laser spectroscopy of atomic beams of short-lived nuclei

    International Nuclear Information System (INIS)

    A possibility of performing laser-nuclear-spectroscopic experiments at qualitatively new level aimed to solve the second-glass current problem and to search T-non invariant effects in the beta-decay of atomic nuclei is discussed. The question of the increase in efficiency of the experiments, aimed to study the main characteristics of nuclei, far from the beta-stability, by means of the laser spectroscopy methods is considered. 147 refs.; 5 figs.; 1 tab

  4. Entanglement generated between a single atom and a laser pulse

    OpenAIRE

    Silberfarb, Andrew; Deutsch, Ivan H.

    2003-01-01

    We quantify the entanglement generated between an atom and a laser pulse in free space. We find that the entanglement calculated using a simple closed-system Jaynes-Cummings Hamiltonian is in remarkable agreement with a full open-system calculation, even though the free-space geometry is far from the strong coupling regime of cavity QED. We explain this result using a simple model in which the atom couples weakly to the laser while coupling strongly to the vacuum. Additionally we place an upp...

  5. Associative ionization of two laser excited Na atoms

    International Nuclear Information System (INIS)

    An investigation into the associative ionization of two sodium atoms excited by polarized laser beams is described. It was possible to excite the Na atoms in a velocity-selective way by exploiting the Doppler effect. The excitation of Na to the 32P3/2, F=3 level is discussed on the basis of so-called saturation curves. Experiments with seven different combinations of polarization of the two exciting laser beams are described and the results discussed. 86 refs.; 53 figs.; 6 tabs

  6. Ionization of atoms by lasers and electric fields

    International Nuclear Information System (INIS)

    A ring dye laser was monitored 5890 A line by a sodium fluorescence cell. The laser was orthogonally directed to interact with a sodium effusive atomic beam. Light radiation from a lamp shifted the excited sodium to near continuum level. The highly excited states are more susceptible to an external field, thus shifting the highly external atoms to the continuum level. The interaction of the electric field causes an increase of two orders of magnitude as compared to two photonionization only. The high signal recorded was due to the probability of the ionization cross section approaching the excited cross section which is several orders of magnitude higher

  7. Laser sources for precision spectroscopy on atomic strontium.

    Science.gov (United States)

    Poli, N; Ferrari, G; Prevedelli, M; Sorrentino, F; Drullinger, R E; Tino, G M

    2006-04-01

    We present a new laser setup designed for high-precision spectroscopy on laser cooled atomic strontium. The system, which is entirely based on semiconductor laser sources, delivers 200 mW at 461 nm for cooling and trapping atomic strontium from a thermal source, 4 mW at 497 nm for optical pumping from the metastable P23 state, 12 mW at 689 nm on linewidth less than 1 kHz for second-stage cooling of the atomic sample down to the recoil limit, 1.2 W at 922 nm for optical trapping close to the "magic wavelength" for the 0-1 intercombination line at 689 nm. The 689 nm laser was already employed to perform a frequency measurement of the 0-1 intercombination line with a relative accuracy of 2.3 x 10(-11), and the ensemble of laser sources allowed the loading in a conservative dipole trap of multi-isotopes strontium mixtures. The simple and compact setup developed represents one of the first steps towards the realization of a transportable optical standards referenced to atomic strontium. PMID:16527534

  8. High energy neutral atoms from high intensity laser plasma interaction

    International Nuclear Information System (INIS)

    Interaction of a high intensity laser with solid targets leads to acceleration of ions from the surface of the target. Ion acceleration is governed by electron dynamics at the target vacuum interface setting up a charge separation. This electron cloud near the target interface can also provide a neutralizing background for ions that have been accelerated. The accelerated ions are thus detected as a high energy neutral atom on a detector. Further, due to the inherent contrast profile of high intensity lasers a pre-plasma is almost always formed and neutral atoms can be detected. The ion and neutral atom energies are measured by a Thomson parabola spectrometer coupled with a 'time of flight' measurement. The neutral atom energies are obtained from the time of flight. The TIFR 20TW laser with an intensity contrast 10-5 was used to carry out the experiment. Defocusing the target led to a 2 fold increase in the neutral atom yield suggesting the role of the pre-plasma. Using a high contrast laser we attempt to tune the recombination dynamics for efficient neutralization of ions by using a controlled pre-plasma. (author)

  9. Determination of mercury by intermittent flow electrochemical cold vapor generation coupled to atomic fluorescence spectrometry

    International Nuclear Information System (INIS)

    A novel method for determination of mercury was developed using an intermittent flow electrochemical cold vapor generation coupled to atomic fluorescence spectrometry (IF-ECVG-AFS). The mercury vapor was generated on the surface of glassy carbon cathode in the flow cell. The operating conditions for the electrochemical generation of mercury vapor were investigated in detail, and the interferences from various ions were evaluated. Under the optimized conditions, no evident memory effects of mercury were observed. The calibration curve was linear up to 5 μg L-1 Hg at 0.54 A cm-2. A detection limit of 1.2 ng L-1 Hg and a relative standard deviation of 1.8% for 1 μg L-1 Hg were obtained. The accuracy of method was verified by the determination of mercury in the certified reference human hair. The ECVG avoided the use of reductants, thereby greatly reducing the contamination sources. In addition, the manifold of IF-ECVG-AFS was simple and amenable to automation

  10. Ablation of biological tissues by radiation of strontium vapor laser

    International Nuclear Information System (INIS)

    A two-stage laser system consisting of a master oscillator and a power amplifier based on sources of self- contained transitions in pairs SrI and SrII has been developed. The radiation spectrum contains 8 laser lines generating in the range of 1 – 6.45 μm, with a generation pulse length of 50 – 150 ns, and pulse energy of ∼ 2.5 mJ. The divergence of the output beam was close to the diffraction and did not exceed 0.5 mrad. The control range of the laser pulse repetition rate varied from 10 to 15 000 Hz. The given laser system has allowed to perform ablation of bone tissue samples without visible thermal damage

  11. Ablation of biological tissues by radiation of strontium vapor laser

    Science.gov (United States)

    Soldatov, A. N.; Vasilieva, A. V.

    2015-11-01

    A two-stage laser system consisting of a master oscillator and a power amplifier based on sources of self- contained transitions in pairs SrI and SrII has been developed. The radiation spectrum contains 8 laser lines generating in the range of 1 - 6.45 μm, with a generation pulse length of 50 - 150 ns, and pulse energy of ˜ 2.5 mJ. The divergence of the output beam was close to the diffraction and did not exceed 0.5 mrad. The control range of the laser pulse repetition rate varied from 10 to 15 000 Hz. The given laser system has allowed to perform ablation of bone tissue samples without visible thermal damage.

  12. Micro-ablation with high power pulsed copper vapor lasers.

    Science.gov (United States)

    Knowles, M

    2000-07-17

    Visible and UV lasers with nanosecond pulse durations, diffraction-limited beam quality and high pulse repetition rates have demonstrated micro-ablation in a wide variety of materials with sub-micron precision and sub-micron-sized heat-affected zones. The copper vapour laser (CVL) is one of the important industrial lasers for micro-ablation applications. Manufacturing applications for the CVL include orifice drilling in fuel injection components and inkjet printers, micro-milling of micromoulds, via hole drilling in printed circuit boards and silicon machining. Recent advances in higher power (100W visible, 5W UV), diffraction-limited, compact CVLs are opening new possibilities for manufacturing with this class of nanosecond laser. PMID:19404369

  13. Ablation of biological tissues by radiation of strontium vapor laser

    Energy Technology Data Exchange (ETDEWEB)

    Soldatov, A. N., E-mail: general@tic.tsu.ru; Vasilieva, A. V., E-mail: anita-tomsk@mail.ru [National Research Tomsk State University, Lenin ave., 36, 634050, Tomsk (Russian Federation)

    2015-11-17

    A two-stage laser system consisting of a master oscillator and a power amplifier based on sources of self- contained transitions in pairs SrI and SrII has been developed. The radiation spectrum contains 8 laser lines generating in the range of 1 – 6.45 μm, with a generation pulse length of 50 – 150 ns, and pulse energy of ∼ 2.5 mJ. The divergence of the output beam was close to the diffraction and did not exceed 0.5 mrad. The control range of the laser pulse repetition rate varied from 10 to 15 000 Hz. The given laser system has allowed to perform ablation of bone tissue samples without visible thermal damage.

  14. Multi-wavelength metal vapor laser systems for solving applied problems of atmospheric spectroscopy

    Science.gov (United States)

    Soldatov, A. N.; Mirza, S. Y.; Polunin, Yu. P.; Shumeiko, A. S.; Kostadinov, I. K.

    2015-11-01

    Results of a cycle of experimental investigations of a multi-wavelength metal vapor laser system based on original configuration of a multi-medium metal vapor laser source are presented. Novelty of our approach consists in that two gas-discharge active elements (on copper bromide and strontium vapors) are arranged in a common cavity, and each of them is pumped by an independent power supply unit, which allows them to be optimized independently for excitation conditions and thereby the output set of lasing wavelengths and their relative power distribution to be regulated. This makes the above-described system promising for a number of scientific and technological applications. The total output power of 11 spectral components lying in the range 0.43-6.45 μm reached ~17 W.

  15. Description of a laser vaporization source and a supersonic cluster beam apparatus

    International Nuclear Information System (INIS)

    Laser vaporization of an appropriate target and recent developments in molecular beam technology have now made it possible to produce supersonic cluster beams of virtually any element in the periodic table. This paper describes the design and principles of a cluster source combined with a time of flight mass spectrometer built for reaction experiments and spectroscopic investigations at Stockholm University

  16. Polymer-coated vertical-cavity surface-emitting laser diode vapor sensor

    DEFF Research Database (Denmark)

    Ansbæk, Thor; Nielsen, Claus Højgaard; Larsen, Niels Bent;

    2010-01-01

    We report a new method for monitoring vapor concentration of volatile organic compounds using a vertical-cavity surface-emitting laser (VCSEL). The VCSEL is coated with a polymer thin film on the top distributed Bragg reflector (DBR). The analyte absorption is transduced to the electrical domain ...

  17. Sub-Doppler laser cooling of potassium atoms

    CERN Document Server

    Landini, M; Carcagni', L; Trypogeorgos, D; Fattori, M; Inguscio, M; Modugno, G

    2011-01-01

    We investigate sub-Doppler laser cooling of bosonic potassium isotopes, whose small hyperfine splitting has so far prevented cooling below the Doppler temperature. We find instead that the combination of a dark optical molasses scheme that naturally arises in this kind of systems and an adiabatic ramping of the laser parameters allows to reach sub-Doppler temperatures for small laser detunings. We demonstrate temperatures as low as 25(3)microK and 47(5)microK in high-density samples of the two isotopes 39K and 41K, respectively. Our findings will find application to other atomic systems.

  18. Sub-Doppler laser cooling of potassium atoms

    Energy Technology Data Exchange (ETDEWEB)

    Landini, M. [LENS and Dipartimento di Fisica e Astronomia, Universita di Firenze, I-50019 Sesto Fiorentino (Italy); INFN, Sezione di Firenze, I-50019 Sesto Fiorentino (Italy); Dipartimento di fisica, Universita di Trento, I-38123 Povo (Trento) (Italy); Roy, S.; Carcagni, L.; Trypogeorgos, D. [LENS and Dipartimento di Fisica e Astronomia, Universita di Firenze, I-50019 Sesto Fiorentino (Italy); Fattori, M.; Inguscio, M.; Modugno, G. [LENS and Dipartimento di Fisica e Astronomia, Universita di Firenze, I-50019 Sesto Fiorentino (Italy); INFN, Sezione di Firenze, I-50019 Sesto Fiorentino (Italy)

    2011-10-15

    We investigate the sub-Doppler laser cooling of bosonic potassium isotopes, whose small hyperfine splitting has so far prevented cooling below the Doppler temperature. We find instead that the combination of a dark optical molasses scheme that naturally arises in this kind of system and an adiabatic ramping of the laser parameters allows us to reach sub-Doppler temperatures for small laser detunings. We demonstrate temperatures as low as 25{+-}3 {mu}K and 47{+-}5 {mu}K in high-density samples of the two isotopes {sup 39}K and {sup 41}K, respectively. Our findings should find application to other atomic systems.

  19. Laser sources for precision spectroscopy on atomic strontium

    OpenAIRE

    Ferrari, G; T.M. Brzozowski; R. DRULLINGER; Poli, N.; Prevedelli, M.; Toninelli, C.; Tino, G. M.

    2004-01-01

    Laser Optics 2003: Solid State Lasers and Nonlinear Frequency Conversion, edited by Vladimir I. Ustugov abstract: We present a new laser setup suited for high precision spectroscopy on atomic strontium. The source is used for an absolute frequency measurement of the visible 5s21S0-5s5p3P1 intercombination line of strontium which is considered a possible candidate for a future optical frequency standard. The optical frequency is measured with an optical comb generator referenced to the SI t...

  20. Formation and Transport of Atomic Hydrogen in Hot-Filament Chemical Vapor Deposition Reactors

    Institute of Scientific and Technical Information of China (English)

    2003-01-01

    In this paper we focus on diamond film hot-filament chemical vapor deposition reactors where the only reactant ishydrogen so as to study the formation and transport of hydrogen atoms. Analysis of dimensionless numbers forheat and mass transfer reveals that thermal conduction and diffusion are the dominant mechanisms for gas-phaseheat and mass transfer, respectively. A simplified model has been established to simulate gas-phase temperature andH concentration distributions between the filament and the substrate. Examination of the relative importance ofhomogeneous and heterogeneous production of H atoms indicates that filament-surface decomposition of molecularhydrogen is the dominant source of H and gas-phase reaction plays a negligible role. The filament-surface dissociationrates of H2 for various filament temperatures were calculated to match H-atom concentrations observed in the liter-ature or derived from power consumption by filaments. Arrhenius plots of the filament-surface hydrogen dissociationrates suggest that dissociation of H2 at refractory filament surface is a catalytic process, which has a rather lowereffective activation energy than homogeneous thermal dissociation. Atomic hydrogen, acting as an important heattransfer medium to heat the substrate, can freely diffuse from the filament to the substrate without recombination.

  1. Search for a permanent EDM with laser cooled radioactive atom

    Science.gov (United States)

    Sakemi, Yasuhiro

    2014-09-01

    To explore the mechanism for the generation of the matter-antimatter asymmetry in the universe, the study on fundamental symmetry violation using the trapped radioactive atoms with laser cooling techniques is being promoted. An Electric Dipole Moment (EDM) of the elementary particle is a good prove to observe the phenomena beyond the Standard Model. A finite value of EDM means the violation of the time reversal symmetry, and the CP violation under the CPT invariance. In paramagnetic atoms, an electron EDM results in an atomic EDM enhanced by the factor of the 3rd power of the charge of the nucleus due the relativistic effects. A heaviest alkali element francium (Fr), which is the radioactive atom, has the largest enhancement factor K ~ 895 in atomic system. Then, we are developing a high intensity laser cooled Fr factory at Cyclotron and Radioisotope Center (CYRIC), Tohoku University to search for the EDM of Fr with the accuracy of 10-29 e cm. To overcome the current accuracy limit of the EDM, it is necessary to realize the high intensity Fr source and to reduce the systematic error due to the motional magnetic field and inhomogeneous applied field. To reduce the dominant component of the systematic errors mentioned above, we will confine the Fr atoms in the small region with the Magneto-Optical Trap (MOT) and optical lattice using the laser cooling and trapping techniques. The construction of the experimental apparatus is making progress, and the new thermal ionizer already produces the Fr of ~ 10 6 ions/s with the primary beam intensity 200 nA. The extracted Fr ion beam is transported to the neutralizer, which is located 10 m downstream, and the produced neutral Fr atoms are introduced into the MOT to load the next trapping system such as the optical dipole force trap and optical lattice. The coherence time will be increased in the laser trapping system, and the present status of the experiment will be reported.

  2. Atoms and molecules interacting with light atomic physics for the laser era

    CERN Document Server

    Straten, Peter van der

    2016-01-01

    This in-depth textbook with a focus on atom-light interactions prepares students for research in a fast-growing and dynamic field. Intended to accompany the laser-induced revolution in atomic physics, it is a comprehensive text for the emerging era in atomic, molecular and optical science. Utilising an intuitive and physical approach, the text describes two-level atom transitions, including appendices on Ramsey spectroscopy, adiabatic rapid passage and entanglement. With a unique focus on optical interactions, the authors present multi-level atomic transitions with dipole selection rules, and M1/E2 and multiphoton transitions. Conventional structure topics are discussed in some detail, beginning with the hydrogen atom and these are interspersed with material rarely found in textbooks such as intuitive descriptions of quantum defects. The final chapters examine modern applications and include many references to current research literature. The numerous exercises and multiple appendices throughout enable advanc...

  3. Guiding cold atoms in a hollow laser beam

    Science.gov (United States)

    Xu, Xinye; Minogin, V. G.; Lee, Kwanil; Wang, Yuzhu; Jhe, Wonho

    1999-12-01

    The theory of atom guiding in a far blue-detuned hollow laser beam (HLB) is developed for the dipole interaction scheme described by a three-level Λ model. The complete kinetic description of atomic motion based on the Fokker-Planck equation for the atomic distribution function is presented. The dipole gradient force, radiation pressure force, and momentum diffusion tensor are then derived. It is found that even for a far-detuned laser beam, the optical potential for a three-level Λ atom is not generally reduced to a sum of two independent potentials associated with the two two-level interactions in the Λ scheme. The theory developed here is also compared with the experimental guiding of cold 85Rb atoms in the HLB. The experimental results are found to be in good agreement with the Monte Carlo simulations based on the three-level Λ model. We observe that the guiding efficiency depends strongly on the intensity and the detuning of the HLB and the initial temperature of atoms. In particular, the experimental results show that, at small detunings, the guiding efficiency is deteriorated strongly by the radiation pressure force. The Monte Carlo simulations also indicate that the efficiency of guiding versus detuning depends strongly on the direction of the HLB propagation with respect to that of atomic motion. Under optimal conditions, the guiding efficiency was found to be about 20%.

  4. Atomic iodine generation via fluorine atoms for chemical oxygen-iodine laser

    Czech Academy of Sciences Publication Activity Database

    Čenský, Miroslav; Špalek, Otomar; Jirásek, Vít; Kodymová, Jarmila; Jakubec, Ivo

    2006-01-01

    Roč. 71, č. 5 (2006), s. 739-755. ISSN 0010-0765 R&D Projects: GA ČR GA202/05/0359; GA ČR GP203/02/D061 Grant ostatní: USAF EOARD(US) FA8655-02-M4040 Institutional research plan: CEZ:AV0Z10100523; CEZ:AV0Z40320502 Keywords : atomic iodine * atomic fluorine * chemical oxygen-iodine laser * COIL Subject RIV: BH - Optics, Masers, Lasers Impact factor: 0.881, year: 2006

  5. Space Debris-de-Orbiting by Vaporization Impulse using Short Pulse Laser

    Energy Technology Data Exchange (ETDEWEB)

    Early, J; Bibeau, C; Claude, P

    2003-09-16

    Space debris constitutes a significant hazard to low earth orbit satellites and particularly to manned spacecraft. A quite small velocity decrease from vaporization impulses is enough to lower the perigee of the debris sufficiently for atmospheric drag to de-orbit the debris. A short pulse (picosecond) laser version of the Orion concept can accomplish this task in several years of operation. The ''Mercury'' short pulse Yb:S-FAP laser being developed at LLNL for laser fusion is appropriate for this task.

  6. Atomic Beam Laser Spectrometer for In-field Isotopic Analysis

    Energy Technology Data Exchange (ETDEWEB)

    Castro, Alonso [Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Actinide Analytical Chemistry Group

    2016-06-22

    This is a powerpoint presentation for the DTRA quarterly program review that goes into detail about the atomic beam laser spectrometer for in-field isotopic analysis. The project goals are the following: analysis of post-detonation debris, determination of U and Pu isotopic composition, and fieldable prototype: < 2ft3, < 1000W.

  7. Scanning laser doppler velocimeter using iodine iodine-vapor discriminator

    International Nuclear Information System (INIS)

    This paper presents a scanning laser doppler velocimeter (SLDV) that is able to measure the velocity over two dimensions. SDV can be used to measure the 2-D velocity of a rotating disk or fluid by using the molecular iodine absorption line (1109) as the frequency discrimination to determine the doppler shift of the target backscattering. The laser source, a narrow line-width Nd:YAG laser at the second harmonic, is frequency locked to the 1109 line as the frequency reference by a digital PID servo with the frequency jitter less than 1 MHz for arbitrarily long periods. Experimental results show that SDV is capable of mapping the speed vector of the target, and the measurement uncertainty of the rotating disk speed is less than 0.25 m/s.

  8. STIRAP in sodium vapor with picosecond laser pulses

    CERN Document Server

    Hicks, Jim L; Allen, Susan D; Tilley, Matt; Hoke, Steven; Johnson, J Bruce

    2015-01-01

    Experimental measurements and calculations of STIRAP transfer efficiencies were made on a sodium gas starting from the $3^2{\\rm S}_{1/2}$ electronic ground state, passing through the $3^2{\\rm P}_{1/2}$ and/or the $3^2{\\rm P}_{3/2}$ to the $5^2{\\rm S}_{1/2}$ state. The lasers used in the experiments had a pulse width of several picoseconds and were close to the Fourier transform limit. Although the linewidth of the laser was much smaller than the spin orbit splitting between the $3^2{\\rm P}_{1/2}$ and $3^2{\\rm P}_{3/2}$ states, Experiments and calculations reveal that both 3p states play a role in the transfer efficiency when the lasers are tuned to resonance through the $3^2{\\rm P}_{1/2}$ state, revealing evidence for quantum interference between the competing pathways.

  9. Influence of laser power on deposition of the chromium atomic beam in laser standing wave

    Institute of Scientific and Technical Information of China (English)

    2009-01-01

    One-dimensional deposition of collimated Cr atomic beam focused by a near-resonant Gaussian standing-laser field with wavelength of 425.55 nm is examined from particle-optics approach by using an adaptive step size,fourth-order Runge-Kutta type algorithm.The influence of laser power on deposition of atoms in laser standing wave is discussed and the simulative result shows that the FWHM of nanometer stripe is 102 nm and contrast is 2:1 with laser power equal to 3 mW,the FWHM is 1.2 nm and contrast is 32:1 with laser power equal to 16 mW,but with laser power increase,equal to 50 mW,the nonmeter structure forms the multi-crests and exacerbates.

  10. Laser and Optical Subsystem for NASA's Cold Atom Laboratory

    Science.gov (United States)

    Kohel, James; Kellogg, James; Elliott, Ethan; Krutzik, Markus; Aveline, David; Thompson, Robert

    2016-05-01

    We describe the design and validation of the laser and optics subsystem for NASA's Cold Atom Laboratory (CAL), a multi-user facility being developed at NASA's Jet Propulsion Laboratory for studies of ultra-cold quantum gases in the microgravity environment of the International Space Station. Ultra-cold atoms will be generated in CAL by employing a combination of laser cooling techniques and evaporative cooling in a microchip-based magnetic trap. Laser cooling and absorption imaging detection of bosonic mixtures of 87 Rb and 39 K or 41 K will be accomplished using a high-power (up to 500 mW ex-fiber), frequency-agile dual wavelength (767 nm and 780 nm) laser and optical subsystem. The CAL laser and optical subsystem also includes the capability to generate high-power multi-frequency optical pulses at 784.87 nm to realize a dual-species Bragg atom interferometer. Currently at Humboldt-Universität zu Berlin.

  11. X-ray refractive index of laser-dressed atoms

    CERN Document Server

    Buth, Christian

    2008-01-01

    We investigated the complex index of refraction in the x-ray regime of atoms in laser light. The laser (intensity up to 10^13 W/cm^2, 800nm) modifies the atomic states but, by assumption, does not excite or ionize the atoms in their electronic ground state. Using quantum electrodynamics, we devise an ab initio theory to calculate the dynamic dipole polarizability and the photoabsorption cross section, which are subsequently used to determine the real and imaginary part, respectively, of the refractive index. The interaction with the laser is treated nonperturbatively; the x-ray interaction is described in terms of a one-photon process. We numerically solve the resolvents involved using a single-vector Lanczos algorithm. Finally, we formulate rate equations to copropagate a laser and an x-ray pulse through a gas cell. Our theory is applied to argon. We study the x-ray polarizability and absorption near the argon K edge over a large range of dressing-laser intensities. We find electromagnetically induced transp...

  12. High sensitivity detection of selenium by laser excited atomic fluorescence spectrometry using electrothermal atomization

    International Nuclear Information System (INIS)

    The high sensitivity detection of the trace element selenium is reported. The analytical method applied is Laser Excited Atomic Fluorescence Spectrometry using Electrothermal Atomization within a graphite furnace atomizer. For the production of tunable laser radiation in the VUV spectral region a laser system was developed which consists of two dye lasers pumped by a Nd:YAG laser. The laser radiations are subsequently frequency doubled and sum frequency mixed by nonlinear optical KDP or BBO crystals, respectively. The system works with a repetition rate of 20 Hz and provides output energies of up to 100 μJ in the VUV at a pulse duration of 5 ns. The analytical investigations were focused on the detection of selenium in aqueous solutions and samples of human whole blood. From measurements on aqueous standards detection limits of 1.5 ng/l for selenium were obtained, with corresponding absolute detected masses of only 15 fg. The linear dynamic range spanned six orders of magnitude and good precision was achieved. In case of human whole blood samples the recovery was found to be within the range of 96% to 104%. The determination of the selenium content yielded medians of [119.5 ± 17.3] μg/l for 200 frozen blood samples taken in 1988 and [109.1 ± 15.6] μg/l for 103 fresh blood samples. (author)

  13. Laser cooling of a magnetically guided ultra cold atom beam

    Energy Technology Data Exchange (ETDEWEB)

    Aghajani-Talesh, Anoush

    2014-07-01

    This thesis examines two complimentary methods for the laser cooling of a magnetically guided ultra-cold atom beam. If combined, these methods could serve as a starting point for high-through put and possibly even continuous production of Bose-Einstein condensates. First, a mechanism is outlined to harvest ultra cold atoms from a magnetically guided atom beam into an optical dipole trap. A continuous loading scheme is described that dissipates the directed kinetic energy of a captured atom via deceleration by a magnetic potential barrier followed by optical pumping to the energetically lowest Zeeman sublevel. The application of this scheme to the transfer of ultra cold chromium atoms from a magnetically guided atom beam into a deep optical dipole trap is investigated via numerical simulations of the loading process. Based on the results of the theoretical studies the feasibility and the efficiency of our loading scheme, including the realisation of a suitable magnetic field configuration, are analysed. Second, experiments were conducted on the transverse laser cooling of a magnetically guided beam of ultra cold chromium atoms. Radial compression by a tapering of the guide is employed to adiabatically heat the beam. Inside the tapered section heat is extracted from the atom beam by a two-dimensional optical molasses perpendicular to it, resulting in a significant increase of atomic phase space density. A magnetic offset field is applied to prevent optical pumping to untrapped states. Our results demonstrate that by a suitable choice of the magnetic offset field, the cooling beam intensity and detuning, atom losses and longitudinal heating can be avoided. Final temperatures below 65 μK have been achieved, corresponding to an increase of phase space density in the guided beam by more than a factor of 30.

  14. Laser cooling of a magnetically guided ultra cold atom beam

    International Nuclear Information System (INIS)

    This thesis examines two complimentary methods for the laser cooling of a magnetically guided ultra-cold atom beam. If combined, these methods could serve as a starting point for high-through put and possibly even continuous production of Bose-Einstein condensates. First, a mechanism is outlined to harvest ultra cold atoms from a magnetically guided atom beam into an optical dipole trap. A continuous loading scheme is described that dissipates the directed kinetic energy of a captured atom via deceleration by a magnetic potential barrier followed by optical pumping to the energetically lowest Zeeman sublevel. The application of this scheme to the transfer of ultra cold chromium atoms from a magnetically guided atom beam into a deep optical dipole trap is investigated via numerical simulations of the loading process. Based on the results of the theoretical studies the feasibility and the efficiency of our loading scheme, including the realisation of a suitable magnetic field configuration, are analysed. Second, experiments were conducted on the transverse laser cooling of a magnetically guided beam of ultra cold chromium atoms. Radial compression by a tapering of the guide is employed to adiabatically heat the beam. Inside the tapered section heat is extracted from the atom beam by a two-dimensional optical molasses perpendicular to it, resulting in a significant increase of atomic phase space density. A magnetic offset field is applied to prevent optical pumping to untrapped states. Our results demonstrate that by a suitable choice of the magnetic offset field, the cooling beam intensity and detuning, atom losses and longitudinal heating can be avoided. Final temperatures below 65 μK have been achieved, corresponding to an increase of phase space density in the guided beam by more than a factor of 30.

  15. Rate-equation approach to atomic-laser light statistics

    International Nuclear Information System (INIS)

    We consider three- and four-level atomic lasers that are either incoherently (unidirectionally) or coherently (bidirectionally) pumped, the single-mode cavity being resonant with the laser transition. The intracavity Fano factor and the photocurrent spectral density are evaluated on the basis of rate equations. According to that approach, fluctuations are caused by jumps in active and detecting atoms. The algebra is simple. Whenever a comparison is made, the expressions obtained coincide with the previous results. The conditions under which the output light exhibits sub-Poissonian statistics are considered in detail. Analytical results, based on linearization, are verified by comparison with Monte Carlo simulations. An essentially exhaustive investigation of sub-Poissonian light generation by three- and four-level lasers has been performed. Only special forms were reported earlier

  16. Hydrogen atom in 2s state in a laser field

    Directory of Open Access Journals (Sweden)

    Vučić Svetlana

    2012-01-01

    Full Text Available The hydrogen atom in the 2s state exposed to a linearly polarized laser field is studied by using the non-perturbative non-Hermitian Floquet theory. The electronic density of the quasi-energy H(2s state versus the electron coordinate is analyzed. We conclude that the decay of an atom in a low-intensity non-resonant laser field occurs from the asymptotically distant part of the initial state. On the other hand, the process of electron emission in a resonant laser field is governed by the excited-bound-statepart of the resonance wave function. With an increase in the intensity and by increasing the degree of excitation of the initial state not too high, the electron is ionized at smaller distances from the nucleus. [Projekat Ministarstva nauke Republike Srbije, br. 171020

  17. CARBON-DIOXIDE LASER VAPORIZATION IN EARLY GLOTTIC CARCINOMA

    NARCIS (Netherlands)

    MAHIEU, HF; PATEL, P; ANNYAS, AA

    1994-01-01

    Objective: Presently, widely employed treatment modalities for early glottic carcinoma include radiation therapy, surgical excision, and carbon dioxide laser excision. All these treatments have good oncological results, but poor or questionable functional-results in terms of quality of voice and muc

  18. Rb atomic magnetometer toward EDM experiment with laser cooled francium atoms

    Science.gov (United States)

    Inoue, Takeshi; Ando, Shun; Aoki, Takahiro; Arikawa, Hiroshi; Harada, Ken-Ichi; Hayamizu, Tomohiro; Ishikawa, Taisuke; Itoh, Masatoshi; Kato, Ko; Kawamura, Hirokazu; Sakamoto, Kosuke; Uchiyama, Aiko; Asahi, Koichiro; Yoshimi, Akihiro; Sakemi, Yasuhiro

    2014-09-01

    A permanent electric dipole moment (EDM) of a particle or an atom is a suited observable to test the physics beyond the standard model. We plan to search for the electron EDM by using the laser cooled francium (Fr) atom, since the Fr atom has a large enhancement factor of the electron EDM and the laser cooling techniques can suppress both statistical and systematic errors. In the EDM experiment, a fluctuation of the magnetic field is a main source of the errors. In order to achieve the high precision magnetometry, a magnetometer based on the nonlinear magneto-optical rotation effect of the Rb atom is under development. A long coherence time of Rb atom is the key issue for the highly sensitive detection of the field fluctuations. The coherence time is limited due both to collisions with an inner surface of a cell contained the Rb atom and to residual field in a magnetic shield. We prepared the cell coated with an anti-relaxation material and measured the relaxation time. A degauss of the shield was performed to eliminate the residual field. We will report the present status of the magnetometer. A permanent electric dipole moment (EDM) of a particle or an atom is a suited observable to test the physics beyond the standard model. We plan to search for the electron EDM by using the laser cooled francium (Fr) atom, since the Fr atom has a large enhancement factor of the electron EDM and the laser cooling techniques can suppress both statistical and systematic errors. In the EDM experiment, a fluctuation of the magnetic field is a main source of the errors. In order to achieve the high precision magnetometry, a magnetometer based on the nonlinear magneto-optical rotation effect of the Rb atom is under development. A long coherence time of Rb atom is the key issue for the highly sensitive detection of the field fluctuations. The coherence time is limited due both to collisions with an inner surface of a cell contained the Rb atom and to residual field in a magnetic shield

  19. High-resolution Resonance Bragg-scattering spectroscopy of an atomic transition from a population difference grating in a vapor cell

    CERN Document Server

    Wang*, Hai; Li, Shujing; Zhang, Chunhong; Xie, Changde; Peng, Kunchi

    2009-01-01

    The laser spectroscopy with a narrow linewidth and high signal to noise ratio (S/N) is very important in the precise measurement of optical frequencies. Here, we present a novel high-resolution backward resonance Bragg-scattering (RBS) spectroscopy from a population difference grating (PDG). The PDG is formed by a standing-wave (SW) pump field in thermal 87Rb vapor, which periodically modulates the space population distribution of two levels in the 87Rb D1 line. A probe beam, having the identical frequency and the orthogonal polarization with the SW pump field, is Bragg-scattered by the PDG. Such Bragg-scattered light becomes stronger at an atomic resonance transition, which forms the RBS spectrum with a high S/N and sub-natural linewidth. Using the scheme of the coherent superposition of the individual Rayleigh-scattered light emitted from the atomic dipole oscillators on the PDG, the experimentally observed RBS spectroscopy is theoretically explained.

  20. Multi-V-type and Λ-type electromagnetically induced transparency experiments in rubidium atoms with low-power low-cost free running single mode diode lasers

    Science.gov (United States)

    Lavín Varela, S.; León Suazo, J. A.; Gutierrez González, J.; Vargas Roco, J.; Buberl, T.; Aguirre Gómez, J. G.

    2016-05-01

    In this work we present the experimental realization of electromagnetically induced transparency (EIT) in A-type and multi-V-type configurations in a sample of rubidium atoms inside a vapor cell at room temperature. Typical EIT windows are clearly visible in the Doppler- broadened absorption signal of the weak probe beam. The coherent optical pump and probe fields are produced by two tunable low-cost, low-power, continuous-wave (cw), free-running and single mode operated diode laser systems, temperature stabilized and current controlled, tuned to the D2 line of rubidium atoms at 780.2 nm wavelength. The continuum wave and single mode operation of our laser systems are confirmed by direct and saturated absorption spectroscopy techniques. Among other applications, these simple experiments can be used as a low-cost undergraduate laboratory in atomic physics, laser physics, coherent light-atom interaction, and high resolution atomic spectroscopy.

  1. Laser remote sensing of water vapor: Raman lidar development

    International Nuclear Information System (INIS)

    The goal of this research is the development of a critical design for a Raman lidar system optimized to match ARM Program needs for profiling atmospheric water vapor at CART sites. This work has emphasized the development of enhanced daytime capabilities using Raman lidar techniques. This abstract touches briefly on the main components of the research program, summarizing results of the efforts. A detailed Raman lidar instrument model has been developed to predict the daytime and nighttime performance capabilities of Raman lidar systems. The model simulates key characteristics of the lidar system, using realistic atmospheric profiles, modeled background sky radiance, and lidar system parameters based on current instrument capabilities. The model is used to guide development of lidar systems based on both the solar-blind concept and the narrowband, narrow field-of-view concept for daytime optimization

  2. Nonadiabatic tunneling ionization of atoms in elliptically polarized laser fields

    International Nuclear Information System (INIS)

    We theoretically investigate the nonadiabatic effects in strong field tunneling ionization of atoms in elliptically polarized laser fields by solving the 3D time-dependent Schrödinger equation (TDSE). Comparing our TDSE results with those of two semi-classical methods, i.e., the quantum-trajectory Monte Carlo simulation (QTMC) and the Coulomb-corrected strong field approximation (CCSFA), we confirm the existence of the nonadiabatic effects with its fingerprint in the nonzero initial lateral velocity at the tunneling exit in the laser polarization plane. Our study shows that these nonadiabatic initial lateral momentum effects become significant in high ellipticity or circularly polarized laser field. These results indicate that the calibration of the experimental laser intensity in this situation should be performed nonadiabatically, which may strongly affect the results of the real tunneling time delay measurements. (paper)

  3. Theoretical femtosecond physics atoms and molecules in strong laser fields

    CERN Document Server

    Grossmann, Frank

    2013-01-01

    Theoretical investigations of atoms and molecules interacting with pulsed or continuous wave lasers up to atomic field strengths on the order of 10^16 W/cm² are leading to an understanding of many challenging experimental discoveries. This book deals with the basics of femtosecond physics and goes up to the latest applications of new phenomena. The book presents an introduction to laser physics with mode-locking and pulsed laser operation. The solution of the time-dependent Schrödinger equation is discussed both analytically and numerically. The basis for the non-perturbative treatment of laser-matter interaction in the book is the numerical solution of the time-dependent Schrödinger equation. The light field is treated classically, and different possible gauges are discussed. Physical phenonema, ranging from Rabi-oscillations in two-level systems to the ionization of atoms, the generation of high harmonics, the ionization and dissociation of molecules as well as the control of chemical reactions are pre...

  4. Injection locking of a high power ultraviolet laser diode for laser cooling of ytterbium atoms

    International Nuclear Information System (INIS)

    We developed a high-power laser system at a wavelength of 399 nm for laser cooling of ytterbium atoms with ultraviolet laser diodes. The system is composed of an external cavity laser diode providing frequency stabilized output at a power of 40 mW and another laser diode for amplifying the laser power up to 220 mW by injection locking. The systematic method for optimization of our injection locking can also be applied to high power light sources at any other wavelengths. Our system does not depend on complex nonlinear frequency-doubling and can be made compact, which will be useful for providing light sources for laser cooling experiments including transportable optical lattice clocks

  5. Performance of a prototype atomic clock based on lin||lin coherent population trapping resonances in Rb atomic vapor

    CERN Document Server

    Mikhailov, Eugeniy E; Belcher, Nathan; Novikova, Irina

    2009-01-01

    We report on the performance of the first table-top prototype atomic clock based on coherent population trapping (CPT) resonances with parallel linearly polarized optical fields (lin||lin configuration). Our apparatus uses a vertical cavity surface emitting laser (VCSEL) tuned to the D1 line of 87Rb with current modulation at the 87Rb hyperfine frequency. We demonstrate cancellation of the first-order light shift by proper choice of rf modulation power, and further improve our prototype clock stability by optimizing the parameters of the microwave lock loop. Operating in these optimal conditions, we measured a short-term fractional frequency stability (Allan deviation) 2*10^{-11} tau^{-1/2} for observation times 1s

  6. Mesoscale imperfections in MoS2 atomic layers grown by a vapor transport technique.

    Science.gov (United States)

    Liu, Yingnan; Ghosh, Rudresh; Wu, Di; Ismach, Ariel; Ruoff, Rodney; Lai, Keji

    2014-08-13

    The success of isolating small flakes of atomically thin layers through mechanical exfoliation has triggered enormous research interest in graphene and other two-dimensional materials. For device applications, however, controlled large-area synthesis of highly crystalline monolayers with a low density of electronically active defects is imperative. Here, we demonstrate the electrical imaging of dendritic ad-layers and grain boundaries in monolayer molybdenum disulfide (MoS2) grown by a vapor transport technique using microwave impedance microscopy. The micrometer-sized precipitates in our films, which appear as a second layer of MoS2 in conventional height and optical measurements, show ∼ 2 orders of magnitude higher conductivity than that of the single layer. The zigzag grain boundaries, on the other hand, are shown to be more resistive than the crystalline grains, consistent with previous studies. Our ability to map the local electrical properties in a rapid and nondestructive manner is highly desirable for optimizing the growth process of large-scale MoS2 atomic layers. PMID:25019334

  7. Synthesis of multiferroic Er-Fe-O thin films by atomic layer and chemical vapor deposition

    Energy Technology Data Exchange (ETDEWEB)

    Mantovan, R., E-mail: roberto.mantovan@mdm.imm.cnr.it; Vangelista, S.; Wiemer, C.; Lamperti, A.; Tallarida, G. [Laboratorio MDM IMM-CNR, I-20864 Agrate Brianza (MB) (Italy); Chikoidze, E.; Dumont, Y. [GEMaC, Université de Versailles St. Quentin en Yvelines-CNRS, Versailles (France); Fanciulli, M. [Laboratorio MDM IMM-CNR, I-20864 Agrate Brianza (MB) (Italy); Dipartimento di Scienza dei Materiali, Università di Milano Bicocca, Milano (Italy)

    2014-05-07

    R-Fe-O (R = rare earth) compounds have recently attracted high interest as potential new multiferroic materials. Here, we report a method based on the solid-state reaction between Er{sub 2}O{sub 3} and Fe layers, respectively grown by atomic layer deposition and chemical vapor deposition, to synthesize Er-Fe-O thin films. The reaction is induced by thermal annealing and evolution of the formed phases is followed by in situ grazing incidence X-ray diffraction. Dominant ErFeO{sub 3} and ErFe{sub 2}O{sub 4} phases develop following subsequent thermal annealing processes at 850 °C in air and N{sub 2}. Structural, chemical, and morphological characterization of the layers are conducted through X-ray diffraction and reflectivity, time-of-flight secondary ion-mass spectrometry, and atomic force microscopy. Magnetic properties are evaluated by magnetic force microscopy, conversion electron Mössbauer spectroscopy, and vibrating sample magnetometer, being consistent with the presence of the phases identified by X-ray diffraction. Our results constitute a first step toward the use of cost-effective chemical methods for the synthesis of this class of multiferroic thin films.

  8. Kinetics of laser-pulse vaporization of uranium carbide by mass spectrometry

    International Nuclear Information System (INIS)

    The kinetics of uranium carbide vaporization in the temperature range 3000 K to 5200 K was studied using a Nd-glass laser with peak power densities from 1.6 x 105 to 4.0 x 105 watts/cm2. The vapor species U, UC2, C1 and C3 were detected and analyzed by a quadrupole mass spectrometer. From the mass spectrometer signals number densities of the various species in the ionizer were obtained as functions of time. The surface of the irradiated uranium carbide was examined by scanning electron microscope and the depth profile of the crater was obtained. In order to aid analysis of the data, the heat conduction and species diffusion equations for the solid (or liquid) were solved numerically by a computer code to obtain the temperature and composition transients during laser heating. A sensitivity analysis was used to study the effect of uncertainties in the input parameters on the computed surface temperatures

  9. Unitary model for atomic ionization by intense XUV laser pulses

    CERN Document Server

    Bustamante, M G

    2016-01-01

    A unitary model describing the electronic transitions in an atom subject to a strong high frequency laser pulse is proposed. The model fully accounts for the initial state coupling with the continuum spectrum. Continuum-continuum as well as discrete-discrete transitions are neglected. The model leads to a single integro-differential equation for the initial state amplitude. Exact numerical and approximate closed semi-analytical solutions of this equation are obtained. A comparison of present results with full time dependent Schr\\"odinger equation solution for Hydrogen atoms subject to a laser pulse is presented. The initial state time dependent population is rather well described by the model and two approximate solutions. The electron energy spectrum is also well reproduced by the model and by a new improved Weiskopf-Wigner related approximation.

  10. Optical emission spectroscopy of metal vapor dominated laser-arc hybrid welding plasma

    International Nuclear Information System (INIS)

    During laser-arc hybrid welding, plasma properties affect the welding process and the weld quality. However, hybrid welding plasmas have not been systematically studied. Here we examine electron temperatures, species densities, and electrical conductivity for laser, arc, and laser-arc hybrid welding using optical emission spectroscopy. The effects of arc currents and heat source separation distances were examined because these parameters significantly affect weld quality. Time-average plasma electron temperatures, electron and ion densities, electrical conductivity, and arc stability decrease with increasing heat source separation distance during hybrid welding. Heat source separation distance affects these properties more significantly than the arc current within the range of currents considered. Improved arc stability and higher electrical conductivity of the hybrid welding plasma result from increased heat flux, electron temperatures, electron density, and metal vapor concentrations relative to arc or laser welding.

  11. Influence of the virtual photon field on the squeezing properties of an atom laser

    Institute of Scientific and Technical Information of China (English)

    Zhao Jian-Gang; Sun Chang-Yong; Wen Ling-Hua; Liang Bao-Long

    2009-01-01

    This paper investigates the squeezing properties of an atom laser without rotating-wave approximation in the system of a binomial states field interacting with a two-level atomic Bose-Einstein condensate. It discusses the influences of atomic eigenfrequency, the interaction intensity between the optical field and atoms, parameter of the binomial states field and virtual photon field on the squeezing properties. The results show that two quadrature components of an atom laser can be squeezed periodically. The duration and the degree of squeezing an atom laser have something to do with the atomic eigenfrequency and the parameter of the binomial states field, respectively. The collapse and revival frequency of atom laser fluctuation depends on the interaction intensity between the optical field and atoms. The effect of the virtual photon field deepens the depth of squeezing an atom laser.

  12. A Simplified Digestion Protocol for the Analysis of Hg in Fish by Cold Vapor Atomic Absorption Spectroscopy

    Science.gov (United States)

    Kristian, Kathleen E.; Friedbauer, Scott; Kabashi, Donika; Ferencz, Kristen M.; Barajas, Jennifer C.; O'Brien, Kelly

    2015-01-01

    Analysis of mercury in fish is an interesting problem with the potential to motivate students in chemistry laboratory courses. The recommended method for mercury analysis in fish is cold vapor atomic absorption spectroscopy (CVAAS), which requires homogeneous analyte solutions, typically prepared by acid digestion. Previously published digestion…

  13. Effect of Laser Power on Atom Probe Tomography of Silicates

    Science.gov (United States)

    Parman, S. W.; Gorman, B.; Jackson, C.; Cooper, R. F.; Diercks, D.

    2011-12-01

    Atom probe tomography (APT) is an emerging analytical method that has the potential to produce nm-scale spatial resolution of atom positions with ppm-level detection limits. Until recently, APT has been limited to analysis of conducting samples due to the high pulsed electrical fields previously required. The recent development of laser-assisted APT now allows much lower laser powers to be used, opening the door to analysis of geologic minerals. The potential applications are many, ranging from diffusion profiles to the distribution of nano-phases to grain boundary chemical properties. We reported the first analysis of natural olivine using APT last year (Parman et al, 2010). While the spatial resolution was good (nm-scale), the accuracy of the compositional analysis was not. Two of the primary barriers to accurate ion identification in APT are: 1) Specimen overheating - This is caused by the interaction of the laser with the low thermal conductivity insulating specimens. Ions are assumed to have left the surface of the sample at the time the laser is pulsed during the analysis (laser pulse width = 12 ps). If the laser power is too high, the surface remains heated for an appreciable time (greater than 5 ns in some cases) after the laser pulse, causing atoms to field evaporate from the surface well after the laser pulse. Since they hit the detector later than the atoms that were released during the pulse, they are interpreted to be higher mass. Thus overheating appears in the analysis as a smearing of mass/charge peaks to higher mass/charge ratios (thermal tails). For well separated peaks, this is not a substantial problem, but for closely spaced peaks, overheating causes artificial mass interferences. 2) Molecular evaporation or clustering - This is also caused by overheating by the laser. Ideally, atoms are field evaporated individually from the surface of the cylindrical specimen. However, if the absorbed energy is high enough, clusters of atoms will be formed

  14. Modification and simulation of the power supply of a metal vapor laser

    Science.gov (United States)

    Ogorodnikov, D. N.; Trigub, M. V.; Torgaev, S. N.; Vasnev, N. A.; Evtushenko, T. G.

    2016-04-01

    The modification of a power supply circuit used for pumping metal vapor lasers is analyzed. The results of OrCAD simulation of the processes that occur in the power supply are presented. The effect of the capacitance ratio on the charging process of a storage capacitor is described. The mode which provides more time for the recovery of the thyratron is discussed. The results of the development of the small-size high pulse repetition frequency laser with up to 3 W average output power are presented.

  15. Transurethral holmium laser vaporization to the urethral tumour through a ureteroscope

    OpenAIRE

    Li, Aihua; Fang, Wei; Zuo, Xiaoming; Feng ZHANG; Li, Weiwu; Lu, Honghai; Liu, Sikuan; Wang, Hui; Zhang, Binghui

    2014-01-01

    We present 2 cases of urethral cancers: one is recurrent bladder transitional cell carcinoma accompanied by urethral metastatic carcinoma located on the right side of verumontanum, and the other is primary bladder and metastatic urethral adenocarcinoma. The urethral tumour was treated by transurethral holmium laser vaporization to the urethral tumour through a ureteroscope and the bladder tumour was treated with transurethral resection and degeneration of the bladder tumour (TURD-Bt). After t...

  16. Simultaneous detection of potassium, water vapor and temperature with tunable diode laser absorption spectroscopy

    OpenAIRE

    Norén, Edvin

    2015-01-01

    Existing tunable diode laser absorption spectroscopy (TDLAS) sensors for potassium (K) and for water vapor (H2O) and temperature were combined to enable simultaneous measurements in combustion and gasification processes. In-situ real-time detection of the above mentioned combustion parameters will improve the understanding of ash-formation during thermochemical conversion of biomass. Simultaneous measurements facilitate the experimental procedure and decrease the methodological uncertainty in...

  17. Synthesis of Cobalt Oxides Thin Films Fractal Structures by Laser Chemical Vapor Deposition

    Directory of Open Access Journals (Sweden)

    P. Haniam

    2014-01-01

    Full Text Available Thin films of cobalt oxides (CoO and Co3O4 fractal structures have been synthesized by using laser chemical vapor deposition at room temperature and atmospheric pressure. Various factors which affect the density and crystallization of cobalt oxides fractal shapes have been examined. We show that the fractal structures can be described by diffusion-limited aggregation model and discuss a new possibility to control the fractal structures.

  18. Attosecond laser pulse ionization of atoms and molecules

    International Nuclear Information System (INIS)

    Ionization dynamics of atoms and molecules under attosecond laser pulses with various photon energies and peak intensities have been investigated using the Time-Dependent Close-Coupling (TDCC) method. We predict the chirp effects on the triply differential probabilities for the ionized electrons of He produced by 450 and 135 asec pulses. In addition, we shall apply our generalized TDCC method to examine the four-body breakup dynamics of molecular hydrogen induced by these ultrashort pulses.

  19. Cold electron sources using laser-cooled atoms

    Science.gov (United States)

    McCulloch, Andrew J.; Sparkes, Ben M.; Scholten, Robert E.

    2016-08-01

    Since the first observation of electron diffraction in 1927, electrons have been used to probe the structure of matter. High-brightness sources of thermal electrons have recently emerged that are capable of simultaneously providing high spatial resolving power along with ultrafast temporal resolution, however they are yet to demonstrate the holy grail of single-shot diffraction of non-crystalline objects. The development of the cold atom electron source, based around the ionisation of laser cooled atoms, has the potential to contribute to this goal. Electron generation from laser cooled atoms is in its infancy, but in just ten years has moved from a proposal to a source capable of performing single-shot diffraction imaging of crystalline structures. The high brightness, high transverse coherence length, and small energy spread of cold electron sources are also potentially advantageous for applications ranging from seeding of x-ray free-electron lasers and synchrotrons to coherent diffractive imaging and microscopy. In this review we discuss the context which motivates the development of these sources, the operating principles of the source, and recent experimental results. The achievements demonstrated thus far combined with theoretical proposals to alleviate current bottlenecks in development promise a bright future for these sources.

  20. Laser cooling of atoms and impact in theoretical physics

    International Nuclear Information System (INIS)

    Exchange of momentum during resonant interaction of laser radiation with atomic systems can decelerate the atoms and reduce their kinetic temperature. Charged particles can be trapped by using a combination of electric and magnetic fields. The cold ions have no first order Doppler effect. This increases the precision of measurement in high resolution spectroscopy. Collisions with buffer gas atoms in a penning trap cool the cyclotron motion of ions but increase the magnetron radius leading to significant loss of ions in the trap. It has been shown that application of an RF field with frequency equal to the sum of the magnetron and cyclotron frequencies can lead to axialisation of ions thereby increasing the spatial overlap of the ions with the radiation and enhancing the sensitivity. The method has been used for measurement of electronic and nuclear g-factors. The high precision with which g-factors of fundamental particles is measured can be used as a test for results of QED calculations. The new mechanism used for trapping of neutral atoms will be discussed. This method has led to interesting new observations such as quantum jump, atomic fountains and Bose-Einstein condensation. Observation of atomic parity violation experiments have led to the discovery of nuclear anapole moment. (author)

  1. Isotopically selective collinear laser photoionization of accelerated helium atoms

    International Nuclear Information System (INIS)

    Collinear two-step laser photoionization of 3He and 4He isotopes, accelerated to energies of up to 3.9 keV, is described. It is shown that the ionization selectivity in the case of the rare isotope 3He is 106 for a residual-gas pressure of 10-7 Torr in the vacuum system. The sensitivity is limited by collisions that result in the excitation of fast metastable atoms to Rydberg states in the field-free region, and by impact ionization of fast atoms in the region of the ionizer. It is shown that the ionization of helium atoms excited to n3D states occurs along the adiabatic and diabatic channels

  2. Laser-cooled atomic ions as probes of molecular ions

    International Nuclear Information System (INIS)

    Trapped laser-cooled atomic ions are a new tool for understanding cold molecular ions. The atomic ions not only sympathetically cool the molecular ions to millikelvin temperatures, but the bright atomic ion fluorescence can also serve as a detector of both molecular reactions and molecular spectra. We are working towards the detection of single molecular ion spectra by sympathetic heating spectroscopy. Sympathetic heating spectroscopy uses the coupled motion of two trapped ions to measure the spectra of one ion by observing changes in the fluorescence of the other ion. Sympathetic heating spectroscopy is a generalization of quantum logic spectroscopy, but does not require ions in the motional ground state or coherent control of the ion internal states. We have recently demonstrated this technique using two isotopes of Ca+ [Phys. Rev. A, 81, 043428 (2010)]. Limits of the method and potential applications for molecular spectroscopy are discussed

  3. Sum frequency and second harmonics generation of copper vapor laser by nonlinear crystals

    International Nuclear Information System (INIS)

    We have demonstrated sum frequency and second harmonic generation using green (510 nm) and yellow (578 nm) laser light of copper vapor lasers (CVL) by nonlinear crystals of KDP and BBO. The beam patterns of the converted UV laser light become stripe due to the restriction of the acceptance angle of KDP crystal which is estimated to be 1.58 mrad. · cm. Conversion efficiency depends on effective crystal length and focusing condition of fundamental laser beam, and is maximized by a convex lens with the focal length of 555 nm. In sum frequency generation, the temporal delay and the pulse shape of 578 nm laser pulse limit the conversion efficiency. In first second harmonic generation using injection locking CVL oscillator system which can produce low beam divergence fundamental laser beam, the maximum conversion efficiency is 11.2% at the incident power of 75 MW/cm2. The BBO crystal is damaged by the higher incident laser power of over 100 MW/cm2. (author)

  4. Enhancement reagents for simultaneous vapor generation of zinc and cadmium with intermittent flow system coupled to atomic fluorescence spectrometry

    International Nuclear Information System (INIS)

    Simultaneous vapor generation of zinc (Zn) and cadmium (Cd) was evaluated by atomic fluorescence spectrometry coupled with an intermittent flow vapor generation system. Some complexing reagents, surfactant and transition metal ions were respectively tested as enhancement reagents. Experiments showed that an appropriate amount of 8-hydroxyquinoline or phenanthroline and nickel ion simultaneously, effectively improved the vapor generation efficiency of Zn and Cd. The volatile species generation was presumed to be a hydrogenation process interpreting how the enhancement reagents played an important role in vapor generation. Additionally, due to the instability of volatile species, reaction temperature, rapid and sufficient mixing of reagents and rapid separation of the volatile species from liquid phase were also crucial. The method of simultaneous determination of Zn and Cd by intermittent flow vapor generation led to the development of atomic fluorescence spectrometry. The detection limits (3σb) were 1.6 μg l-1 for Zn and 0.01 μg l-1 for Cd and the relative standard deviations were 3.6% for Zn (50 μg l-1, n=11) and 1.7% for Cd (2 μg l-1, n=11) respectively. Results for the determination of Zn and Cd have been confirmed by the analysis of CRMs with good agreement between the certified and found values

  5. Search for a permanent EDM using laser cooled radioactive atom

    International Nuclear Information System (INIS)

    An Electric Dipole Moment (EDM) of the elementary particle is a good prove to observe the phenomena beyond the Standard Model. A non-zero EDM shows the violation of the time reversal symmetry, and under the CPT invariance it means the CP violation. In paramagnetic atoms, an electron EDM results in an atomic EDM enhanced by the factor of the 3rd power of the charge of the nucleus due the relativistic effects. A heaviest alkali element francium (Fr), which is the radioactive atom, has the largest enhancement factor K ∼ 895. Then, we are developing a high intensity laser cooled Fr factory at Cyclotron and Radioisotope Center (CYRIC), Tohoku University to perform the search for the EDM of Fr with the accuracy of 10-29 e · cm. The important points to overcome the current accuracy limit of the EDM are to realize the high intensity Fr source and to reduce the systematic error due to the motional magnetic field and inhomogeneous applied field. To reduce the dominant component of the systematic errors mentioned above, we will confine the Fr atoms in the small region with the Magneto-Optical Trap and optical lattice using the laser cooling and trapping techniques. The construction of the experimental apparatus is making progress, and the new thermal ionizer already produces the Fr of ∼106 ions/s with the primary beam intensity 200 nA. The developments of the laser system and optical equipments are in progress, and the present status and future plan of the experimental project is reported.

  6. Search for a permanent EDM using laser cooled radioactive atom

    Science.gov (United States)

    Sakemi, Y.; Harada, K.; Hayamizu, T.; Itoh, M.; Kawamura, H.; Liu, S.; Nataraj, H. S.; Oikawa, A.; Saito, M.; Sato, T.; Yoshida, H. P.; Aoki, T.; Hatakeyama, A.; Murakami, T.; Imai, K.; Hatanaka, K.; Wakasa, T.; Shimizu, Y.; Uchida, M.

    2011-07-01

    An Electric Dipole Moment (EDM) of the elementary particle is a good prove to observe the phenomena beyond the Standard Model. A non-zero EDM shows the violation of the time reversal symmetry, and under the CPT invariance it means the CP violation. In paramagnetic atoms, an electron EDM results in an atomic EDM enhanced by the factor of the 3rd power of the charge of the nucleus due the relativistic effects. A heaviest alkali element francium (Fr), which is the radioactive atom, has the largest enhancement factor K ~ 895. Then, we are developing a high intensity laser cooled Fr factory at Cyclotron and Radioisotope Center (CYRIC), Tohoku University to perform the search for the EDM of Fr with the accuracy of 10-29 e · cm. The important points to overcome the current accuracy limit of the EDM are to realize the high intensity Fr source and to reduce the systematic error due to the motional magnetic field and inhomogeneous applied field. To reduce the dominant component of the systematic errors mentioned above, we will confine the Fr atoms in the small region with the Magneto-Optical Trap and optical lattice using the laser cooling and trapping techniques. The construction of the experimental apparatus is making progress, and the new thermal ionizer already produces the Fr of ~106 ions/s with the primary beam intensity 200 nA. The developments of the laser system and optical equipments are in progress, and the present status and future plan of the experimental project is reported.

  7. Interaction between laser-induced plasma/vapor and arc plasma during fiber laser-MIG hybrid welding

    International Nuclear Information System (INIS)

    Hybrid plasma is an important physical phenomenon in fiber laser-MIG hybrid welding. It greatly affects the stability of the process, the quality of the weld, and the efficiency of energy coupling. In this paper, clear and direct proofs of these characteristics are presented through high-speed video images. Spectroscopic analysis is used to describe the characterization of hybrid plasma. The hybrid plasma forms a curved channel between the welding wire and the keyhole during the fiber laser-MIG hybrid welding process. The curved channel is composed of two parts. The laser-induced plasma/vapor expands due to the combined effect of the laser and the MIG arc, forming an ionization duct, which is one part of the curved channel. The resistance of the duct is smaller than that of other locations because of the rise in electrical conductivity. Consequently, the electrical arc is guided through the duct to the surface of the material, which is the other part of the curved channel. The spectral intensities of metal elements in laser-MIG hybrid welding are much stronger than those in MIGonly welding, whereas the spectral intensities of shielding gas element in laser-MIG hybrid welding are much weaker

  8. Urethral stricture vaporization with the KTP laser provides evidence for a favorable impact of laser surgery on wound healing

    Science.gov (United States)

    Schmidlin, Franz R.; Venzi, Giordano; Jichlinski, Patrice; Oswald, Michael; Delacretaz, Guy P.; Gabbiani, Giulio; Leisinger, Hans-Juerg; Graber, Peter

    1997-12-01

    The objective of this study was to evaluate and compare the safety and efficacy of the KTP 532 laser to direct vision internal urethrotomy (DVIU) in the management of urethral strictures. A total of 32 patients were randomized prospectively in this study, 14 DVIU and 18 KTP 532 laser. Patients were evaluated postoperatively with flowmetry and in the case of recurrence with cystourethrography at 3, 12, 24 weeks. With the KTP 532 laser complete symptomatic and uredynamic success was achieved in 15 (83%) patients at 12 and 24 weeks. Success rate was lower in the DVIU group with 9 (64%) patients at 12 weeks and 8 (57%) patients at 24 weeks. Mean preoperative peak-flow was improved from 6 cc/s to 20 cc/s at 3, 12 and 24 weeks with the KTP laser. With DVIU mean preoperative peak-flow was improved from 5.5 cc/s to 20 cc/s at 3 weeks followed by a steady decrease to 13 cc/s at 12 weeks and to 12 cc/s 24 weeks. No complication was observed in either group of patients. Our results confirm that stricture vaporization with the KTP 532 laser is a safe and efficient procedure. The better results after laser surgery make it also a valuable alternative in the endoscopic treatment of urethral strictures. These findings suggest a favorable influence of laser surgery on wound healing with less wound contraction and scarring. The lack of contraction of laser wounds might be related to the absence and the lack of organization of myofibroblasts in laser induced lesions.

  9. The Laser Damage Threshold for Materials and the Relation Between Solid-Melt and Melt-Vapor Interface Velocities

    International Nuclear Information System (INIS)

    Numerous experiments have demonstrated and analytic theories have predicted that there is a threshold for pulsed laser ablation of a wide range of materials. Optical surface damage threshold is a very complex and important application of high-power lasers. Optical damage may also be considered to be the initial phase of laser ablation. In this work it was determined the time required and the threshold energy of a layer of thickness to heat up. We used the Finite Difference method to simulate the process of laser-target interaction in three cases. Namely, the case before melting begins using a continuous wave (c.w) laser source and a pulsed laser source, the case after the first change of state (from solid to melt), and the case after the second change of state (from melt to vapor). And also study the relation between the solid-melt and melt-vapor interface velocities to have a commonsense of the laser ablation process.

  10. Laser isotope separation using Ti:sapphire laser

    International Nuclear Information System (INIS)

    The application of Ti:sapphire laser to atomic vapor laser isotope separation is studied. The laser system needs broad tunability, narrow linewidth, high power, high repetition rate, etc. The laser was applied for the laser isotope separation of rubidium. Ion spectra of each isotope indicate that each isotope, 85Rb and 87Rb, was selectively photoionized. (author)

  11. Nuclear-driven flashlamp pumping of the atomic iodine laser

    International Nuclear Information System (INIS)

    This report is a study of the atomic iodine laser pumped with nuclear- excited XeBr fluorescence. Preliminary experiments, conducted in the TRIGA reactor investigated the fluorescence of the excimer XeBr under nuclear pumping with 10B and 3He, for use as a flashlamp gas to stimulate the laser. These measurements included a determination of the fluorescence efficiency (light emitted in the wavelength region of interest, divided by energy deposited in the gas) of XeBr under nuclear pumping, with varying excimer mixtures. Maximum fluorescence efficiencies were approximately 1%. In order to better understand XeBr under nuclear excitation, a kinetics model of the system was prepared. The model generated the time-dependant concentrations of 20 reaction species for three pulse sizes, a TRIGA pulse, a fast burst reactor pulse, and an e-beam pulse. The modeling results predicted fluorescence efficiencies significantly higher (peak efficiencies of approximately 10%) than recorded in the fluorescence experiments. The cause of this discrepancy was not fully determined. A ray tracing computer model was also prepared to evaluate the efficiency with which nuclear-induced fluorescence generated in one cavity of a laser could be coupled into another cavity containing an iodine lasant. Finally, an experimental laser cell was constructed to verify that nuclear-induced XeBr fluorescence could be used to stimulate a laser. Lasing was achieved at 1.31 micron in the TRIGA using C3F7I, a common iodine lasant. Peak laser powers were approximately 20 mW. Measured flashlamp pump powers at threshold agreed well with literature values, as did lasant pressure dependency on laser operation

  12. Near resonant absorption by atoms in intense fluctuating laser fields

    International Nuclear Information System (INIS)

    The objective of this program was to make quantitative measurements of the effects of higher-order phase/frequency correlations in a laser beam on nonlinear optical absorption processes in atoms. The success of this program was due in large part to a unique experimental capability for modulating the extracavity beam of a stabilized (approx-lt 200 kHz) continuous-wave laser with statistically-well-characterized stochastic phase (or frequency) fluctuations, in order to synthesize laser bandwidths to ∼20 MHz (depending on noise amplitude), with profiles variable between Gaussian and Lorentzian (depending on noise bandwidth). Laser driven processes investigated included the following: (1) the optical Autler-Towns effect in the 3S1/2 (F = 2, MF = 2) → 3P3/2 (F = 3, MF = 3) two- level Na resonance, using a weak probe to the 4D5/2 level; (2) the variance and spectra of fluorescence intensity fluctuations in the two-level Na resonance; (3) the Hanle effect in the 1S0 - 3P1, transition at λ = 555.6 nm in 174 Yb; (4) absorption (and gain) of a weak probe, when the probe is a time-delayed replica of the resonant (with the two-level Na transition) pump laser; and (5) four-wave-mixing in a phase-conjugate geometry, in a sodium cell, and, finally, in a diffuse atomic sodium beam. The experimental results from these several studies have provided important confirmation of advanced theoretical methods

  13. Performance of a prototype atomic clock based on lin parallel lin coherent population trapping resonances in Rb atomic vapor

    International Nuclear Information System (INIS)

    We report on the performance of the first table-top prototype atomic clock based on coherent population trapping (CPT) resonances with parallel linearly polarized optical fields (lin parallel lin configuration). Our apparatus uses a vertical-cavity surface-emitting laser (VCSEL) tuned to the D1 line of 87Rb with the current modulation at the 87Rb hyperfine frequency. We demonstrate cancellation of the first-order light shift by the proper choice of rf modulation power and further improve our prototype clock stability by optimizing the parameters of the microwave lock loop. Operating in these optimal conditions, we measured a short-term fractional frequency stability (Allan deviation) 2x10-11τ-1/2 for observation times 1 s≤τ≤20 s. This value is limited by large VCSEL phase noise and environmental temperature fluctuation. Further improvements in frequency stability should be possible with an apparatus designed as a dedicated lin parallel lin CPT resonance clock with environmental impacts minimized.

  14. Laser cooling, trapping, and Rydberg spectroscopy of neutral holmium atoms

    Science.gov (United States)

    Hostetter, James Allen

    This thesis focuses on progress towards using ensembles of neutral holmium for use in quantum computing operations. We are particularly interested in using a switchable interaction between neutral atoms, the Rydberg blockade, to implement a universal set of quantum gates in a collective encoding scheme that presents many benefits over quantum computing schemes which rely on physically distinct qubits. We show that holmium is uniquely suited for operations in a collective encoding basis because it has 128 ground hyperfine states, the largest number of any stable, neutral atom. Holmium is a rare earth atom that is very poorly described for our purposes as it has never been cooled and trapped, its spectrum is largely unknown, and it presents several unique experimental challenges related to its complicated atomic structure and short wavelength transitions. We demonstrate important progress towards overcoming these challenges. We produce the first laser cooling and trapping of holmium into a MOT. Because we use a broad cooling transition, our cooling technique does not require the use of a Zeeman slower. Using MOT depletion spectroscopy, we provide precise measurements of holmium's Rydberg states and its ionization potential. Our work continues towards cooling holmium into a dipole trap by calculating holmium's AC polarizability and demonstrating the results of early attempts at an optical dipole trap. We provide details of future upgrades to the experimental apparatus and discuss interesting potential for using holmium in quantum computing using single atoms in a magnetically trapped lattice. This thesis shows several promising indicators for continued work in this field.

  15. High-speed microjet generation using laser-induced vapor bubbles

    Science.gov (United States)

    Oudalov, Nikolai; Tagawa, Yoshiyuki; Peters, Ivo; Visser, Claas-Willem; van der Meer, Devaraj; Prosperetti, Andrea; Sun, Chao; Lohse, Detlef

    2011-11-01

    The generation and evolution of microjets are studied both experimentally and numerically. The jets are generated by focusing a laser pulse into a microscopic capillary tube (~50 μm) filled with water-based red dye. A vapor bubble is created instantly after shooting the laser (microjet forms. The process of jet formation is captured using high-speed recordings at 1.0 × 106 fps. The velocity of the microjets can reach speeds of ~850 m/s while maintaining a very sharp geometry. The high-speed recordings enable us to study the effect of several parameters on the jet velocity, e.g. the absorbed energy and the distance between the laser spot and the free surface.The results show a clear dependence on these variables, even for supersonic speeds. Comparisons with numerical simulations confirm the nature of these dependencies.

  16. Relationship between 578-nm (copper vapor) laser beam geometry and heat distribution within biological tissues

    Science.gov (United States)

    Ilyasov, Ildar K.; Prikhodko, Constantin V.; Nevorotin, Alexey J.

    1995-01-01

    Monte Carlo (MC) simulation model and the thermoindicative tissue phantom were applied for evaluation of a depth of tissue necrosis (DTN) as a result of quasi-cw copper vapor laser (578 nm) irradiation. It has been shown that incident light focusing angle is essential for DTN. In particular, there was a significant rise in DTN parallel to elevation of this angle up to +20 degree(s)C and +5 degree(s)C for both the MC simulation and tissue phantom models, respectively, with no further increase in the necrosis depth above these angles. It is to be noted that the relationship between focusing angles and DTN values was apparently stronger for the real target compared to the MC-derived hypothetical one. To what extent these date are applicable for medical practice can be evaluated in animal models which would simulate laser-assisted therapy for PWS or related dermatologic lesions with converged 578 nm laser beams.

  17. Differential absorption lidar measurements of atmospheric water vapor using a pseudonoise code modulated AlGaAs laser. Thesis

    Science.gov (United States)

    Rall, Jonathan A. R.

    1994-01-01

    Lidar measurements using pseudonoise code modulated AlGaAs lasers are reported. Horizontal path lidar measurements were made at night to terrestrial targets at ranges of 5 and 13 km with 35 mW of average power and integration times of one second. Cloud and aerosol lidar measurements were made to thin cirrus clouds at 13 km altitude with Rayleigh (molecular) backscatter evident up to 9 km. Average transmitter power was 35 mW and measurement integration time was 20 minutes. An AlGaAs laser was used to characterize spectral properties of water vapor absorption lines at 811.617, 816.024, and 815.769 nm in a multipass absorption cell using derivative spectroscopy techniques. Frequency locking of an AlGaAs laser to a water vapor absorption line was achieved with a laser center frequency stability measured to better than one-fifth of the water vapor Doppler linewidth over several minutes. Differential absorption lidar measurements of atmospheric water vapor were made in both integrated path and range-resolved modes using an externally modulated AlGaAs laser. Mean water vapor number density was estimated from both integrated path and range-resolved DIAL measurements and agreed with measured humidity values to within 6.5 percent and 20 percent, respectively. Error sources were identified and their effects on estimates of water vapor number density calculated.

  18. Determination of mercury by multisyringe flow injection system with cold-vapor atomic absorption spectrometry

    International Nuclear Information System (INIS)

    A new software-controlled time-based multisyringe flow injection system for mercury determination by cold-vapor atomic absorption spectrometry is proposed. Precise known volumes of sample, reducing agent (1.1% SnCl2 in 3% HCl) and carrier (3% HCl) are dispensed into a gas-liquid separation cell with a multisyringe burette coupled with one three-way solenoid valve. An argon flow delivers the reduced mercury to the spectrometer. The optimization of the system was carried out testing reaction coils and gas-liquid separators of different design as well as changing parameters, such as sample and reagents volumes, reagent concentrations and carrier gas flow rate, among others. The analytical curves were obtained within the range 50-5000 ng L-1. The detection limit (3σ b/S) achieved is 5 ng L-1. The relative standard deviation (R.S.D.) was 1.4%, evaluated from 16 successive injections of 250 ng L-1 Hg standard solution. The injection and sample throughput per hour were 44 and 11, respectively. This technique was validated by means of solid and water reference materials with good agreement with the certified values and was successfully applied to fish samples

  19. Delta-doping of boron atoms by photoexcited chemical vapor deposition

    International Nuclear Information System (INIS)

    Boron delta-doped structures in Si crystals were fabricated by means of photoexcited chemical vapor deposition (CVD). Core electronic excitation with high-energy photons ranging from vacuum ultraviolet to soft x rays decomposes B2H6 molecules into fragments. Combined with in situ monitoring by spectroscopic ellipsometry, limited number of boron hydrides can be delivered onto a Si(100) surface by using the incubation period before the formation of a solid boron film. The boron-covered surface is subsequently embedded in a Si cap layer by Si2H6 photo-excited CVD. The crystallinity of the Si cap layer depended on its thickness and the substrate temperature. The evaluation of the boron depth profile by secondary ion mass spectroscopy revealed that boron atoms were confined within the delta-doped layer at a concentration of 2.5 x 1020 cm-3 with a full width at half maximum of less than 9 nm, while the epitaxial growth of a 130-nm-thick Si cap layer was sustained at 420 deg. C.

  20. Elucidating the Structure of Sugars: MW Spectroscopy Combined with Ultrafast UV Laser Vaporization

    Science.gov (United States)

    Cocinero, Emilio J.; Ecija, Patricia; Basterretxea, Francisco J.; Fernandez, Jose A.; Castano, Fernando; Lesarri, Alberto; Grabow, Jens-Uwe; Cimas, Alvaro

    2013-06-01

    Carbohydrates are one of the most versatile biochemicalbuilding blocks, widely acting in energetic, structural or recognition processes. Even the small monosaccharides display unique structural and conformational freedom and may coexist in many open-chain or cyclic forms. We recently initiated the investigation of a series of monosaccharides using a combination of ultrafast laser vaporization and microwave spectroscopy in supersonic jet expansions. We present several structural studies on carbohydrates of aldoses and ketoses of five and six carbon sugars vaporized by UV ultrafast laser vaporization and stabilized in a jet expansion. The experimental evidence confirms that sugars exhibits a α-/β-pyranose conformation (6-membered ring), sharply contrasting with the furanose form (5-membered ring) found in the nature (as component of RNA, sucrose). In addition, thanks to the use of enriched samples, we have experimentally determined the substitution and effective structures. Finally, the structure of several monosaccharides was compared and common structural patterns of their conformational landscape will be showed. E. J. Cocinero, A. Lesarri, P. écija, F. J. Basterretxea, J. U. Grabow, J. A. Fernández and F. Castaño Angew. Chem. Int. Ed. 51, 3119-3124, 2012. E. J. Cocinero, A. Lesarri, P. écija, Á. Cimas, B. G. Davis, F. J. Basterretxea, J. A. Fernández and F. Castaño J. Am. Chem. Soc. 135, 2845-2852, 2013.

  1. Physics of zinc vaporization and plasma absorption during CO2 laser welding

    International Nuclear Information System (INIS)

    A number of mathematical models have been developed earlier for single-material laser welding processes considering one-, two-, and three-dimensional heat and mass transfers. However, modeling of laser welding of materials with multiple compositions has been a difficult problem. This paper addresses a specific case of this problem where CO2 laser welding of zinc-coated steel, commonly used in automobile body manufacturing, is mathematically modeled. The physics of a low boiling point material, zinc, is combined with a single-material (steel) welding model, considering multiple physical phenomena such as keyhole formation, capillary and thermocapillary forces, recoil and vapor pressures, etc. The physics of laser beam-plasma interaction is modeled to understand the effect on the quality of laser processing. Also, an adaptive meshing scheme is incorporated in the model for improving the overall computational efficiency. The model, whose results are found to be in close agreement with the experimental observations, can be easily extended for studying zinc-coated steel welding using other high power, continuous wave lasers such as Nd:YAG and Yb:YAG

  2. Thermal dynamics-based mechanism for intense laser-induced material surface vaporization

    Indian Academy of Sciences (India)

    N Kumar; S Dash; A K Tyagi; Baldev Raj

    2008-09-01

    Laser material processing involving welding, ablation and cutting involves interaction of intense laser pulses of nanosecond duration with a condensed phase. Such interaction involving high brightness radiative flux causes multitude of non-linear events involving thermal phase transition at soild–liquid–gas interfaces. A theoretical perspective involving thermal dynamics of the vaporization process and consequent non-linear multiple thermal phase transitions under the action of laser plasma is the subject matter of the present work. The computational calculations were carried out where titanium (Ti) was treated as a condensed medium. The solution to the partial differential equations governing the thermal dynamics and the underlying phase transition event in the multiphase system is based on non-stationary Eulerian variables. The Mach number depicts significant fluctuations due to thermal instabilities associated with the laser beam flux and intensity. A conclusive amalgamation has been established which relates material surface temperature profile to laser intensity, laser flux and the pressure in the plasma cloud.

  3. Tunable Diode Laser Atomic Absorption Spectroscopy for Detection of Potassium under Optically Thick Conditions.

    Science.gov (United States)

    Qu, Zhechao; Steinvall, Erik; Ghorbani, Ramin; Schmidt, Florian M

    2016-04-01

    Potassium (K) is an important element related to ash and fine-particle formation in biomass combustion processes. In situ measurements of gaseous atomic potassium, K(g), using robust optical absorption techniques can provide valuable insight into the K chemistry. However, for typical parts per billion K(g) concentrations in biomass flames and reactor gases, the product of atomic line strength and absorption path length can give rise to such high absorbance that the sample becomes opaque around the transition line center. We present a tunable diode laser atomic absorption spectroscopy (TDLAAS) methodology that enables accurate, calibration-free species quantification even under optically thick conditions, given that Beer-Lambert's law is valid. Analyte concentration and collisional line shape broadening are simultaneously determined by a least-squares fit of simulated to measured absorption profiles. Method validation measurements of K(g) concentrations in saturated potassium hydroxide vapor in the temperature range 950-1200 K showed excellent agreement with equilibrium calculations, and a dynamic range from 40 pptv cm to 40 ppmv cm. The applicability of the compact TDLAAS sensor is demonstrated by real-time detection of K(g) concentrations close to biomass pellets during atmospheric combustion in a laboratory reactor. PMID:26938713

  4. Ambient Molecular Analysis of Biological Tissue Using Low-Energy, Femtosecond Laser Vaporization and Nanospray Postionization Mass Spectrometry

    Science.gov (United States)

    Shi, Fengjian; Flanigan, Paul M.; Archer, Jieutonne J.; Levis, Robert J.

    2016-03-01

    Direct analysis of plant and animal tissue samples by laser electrospray mass spectrometry (LEMS) was investigated using low-energy, femtosecond duration laser vaporization at wavelengths of 800 and 1042 nm followed by nanospray postionization. Low-energy (optimal cutting temperature compounds that are commonly used in animal tissue cryosections.

  5. Coherence of a squeezed sodium atom laser generated from Raman output coupling

    Institute of Scientific and Technical Information of China (English)

    Huiyong He; Chunjia Huang

    2009-01-01

    The coherence of a squeezed sodium atom laser generated from a Raman output coupler,in which the sodium atoms in Bose-Einstein condensate (BEC) intcract with two light beams consisting of a weaker squeezed coherent probe light and a stronger classical coupling light,is investigated.The results show that in the case of a large mean number of BEC atoms and a weaker probe light field,the atom laser is antibunching,and this atom laser is second-order coherent if the number of BEC atoms in traps is large enough.

  6. Green method for ultrasensitive determination of Hg in natural waters by electrothermal-atomic absorption spectrometry following sono-induced cold vapor generation and 'in-atomizer trapping'

    International Nuclear Information System (INIS)

    Sono-induced cold vapor generation (SI-CVG) has been used for the first time in combination with a graphite furnace atomizer for determination of Hg in natural waters by electrothermal-atomic absorption spectrometry after in situ trapping onto a noble metal-pretreated platform (Pd, Pt or Rh) inserted into a graphite tube. The system allows 'in-atomizer trapping' of Hg without the use of conventional reduction reactions based on sodium borohydride or tin chloride in acid medium for cold vapor generation. The sono-induced reaction is accomplished by applying ultrasound irradiation to the sample solution containing Hg(II) in the presence of an organic compound such as formic acid. As this organic acid is partly degraded upon ultrasound irradiation to yield CO, CO2, H2 and H2O, the amount of lab wastes is minimized and a green methodology is achieved. For this purpose, experimental variables influencing the generation/trapping process are fully investigated. The limit of detection for a 10 min trapping time and 10 mL sample volume was 0.03 μg L-1 (Integrated absorbance) and the repeatability expressed as relative standard deviation was about 3%. Carbonates and chlorides at 100 mg L-1 level caused a signal depression by 20-30%. The enhanced trapping efficiency observed with the sono-induced cold vapor generation as compared with 'in-atomizer trapping' methods employing chemical vapor generation is discussed. A reaction pathway for SI-CVG is proposed on the basis of the current knowledge for synthesis of noble metal nanoparticles by ultrasound

  7. Determination of mercury by electrochemical cold vapor generation atomic fluorescence spectrometry using polyaniline modified graphite electrode as cathode

    Energy Technology Data Exchange (ETDEWEB)

    Jiang Xianjuan [Department of Chemistry, University of Science and Technology of China, Hefei, Anhui 230026 (China); Gan Wuer, E-mail: wgan@ustc.edu.c [Department of Chemistry, University of Science and Technology of China, Hefei, Anhui 230026 (China); Wan Lingzhong; Zhang Hanchang; He Youzhao [Department of Chemistry, University of Science and Technology of China, Hefei, Anhui 230026 (China)

    2010-02-15

    An electrochemical cold vapor generation system with polyaniline modified graphite electrode as cathode material was developed for Hg (II) determination by coupling with atomic fluorescence spectrometry. This electrochemical cold vapor generation system with polyaniline/graphite electrode exhibited higher sensitivity; excellent stability and lower memory effect compared with graphite electrode electrochemical cold vapor generation system. The relative standard deviation was 2.7% for eleven consecutive measurements of 2 ng mL{sup -1} Hg (II) standard solution and the mercury limit of detection for the sample blank solution was 1.3 rg mL{sup -1} (3sigma). The accuracy of the method was evaluated through analysis of the reference materials (GBW09101) (Human hair) and GBW (08517) (Laminaria Japonica Aresch) and the proposed method was successfully applied to the analysis of human hairs.

  8. On-line laser spectroscopy with thermal atomic beams

    CERN Document Server

    Thibault, C; De Saint-Simon, M; Duong, H T; Guimbal, P; Huber, G; Jacquinot, P; Juncar, P; Klapisch, Robert; Liberman, S; Pesnelle, A; Pillet, P; Pinard, J; Serre, J M; Touchard, F; Vialle, J L

    1981-01-01

    On-line high resolution laser spectroscopy experiments have been performed in which the light from a CW tunable dye laser interacts at right angles with a thermal atomic beam. /sup 76-98/Rb, /sup 118-145 /Cs and /sup 208-213/Fr have been studied using the ionic beam delivered by the ISOLDE on-line mass separator at CERN while /sup 30-31/Na and /sup 38-47/K have been studied by setting the apparatus directly on-line with the PS 20 GeV proton beam. The principle of the method is briefly explained and some results concerning nuclear structure are given. The hyperfine structure, spins and isotope shifts of the alkali isotopes and isomers are measured. (8 refs).

  9. Enhanced generation of VUV radiation by four-wave mixing in mercury using pulsed laser vaporization

    CERN Document Server

    Chenais, Sebastien; Philippet, Laurent; Castex, Marie-Claude

    2007-01-01

    The efficiency of a coherent VUV source at 125 nm, based on 2-photon resonant four-wave mixing in mercury vapor, has been enhanced by up to 2 orders of magnitude. This enhancement was obtained by locally heating a liquid Hg surface with a pulsed excimer laser, resulting in a high density vapor plume in which the nonlinear interaction occurred. Energies up to 5 μJ (1 kW peak power) have been achieved while keeping the overall Hg cell at room temperature, avoiding the use of a complex heat pipe. We have observed a strong saturation of the VUV yield when peak power densities of the fundamental beams exceed the GW/cm2 range, as well as a large intensity-dependant broadening (up to ~30 cm-1) of the two-photon resonance. The source has potential applications for high resolution interference lithography and photochemistry.

  10. Enabling Nanotechnology with Focused Ion Beams from Laser Cooled Atoms

    Science.gov (United States)

    Steele, A. V.; Knuffman, B.; Orloff, J.; Maazouz, M.; McClelland, J. J.

    2011-05-01

    The Magneto-Optical Trap Ion Source (MOTIS) being developed at NIST has the potential to enable numerous advances in nanoscale science. In a MOTIS, atoms are captured into a MOT, photoionized, and accelerated to an energy of a few hundred eV to a few tens of kV. A beam formed in this way can be brought to a tight focus, competitive with the commercial focused ion beam machines deployed widely today. Additionally, the unique characteristics of this source, coupled with the user's choice of ion from the long and growing list of laser-coolable atomic species suggest that the MOTIS has the potential to advance the state of the art in applications such as imaging, nanofabrication, secondary ion mass spectrometry, and others. I will present high-resolution images from our lithium and chromium MOTIS-based focused ion beams and discuss applications which we will pursue with these new tools.

  11. Adiabatic theory of ionization of atoms by intense laser pulses

    International Nuclear Information System (INIS)

    As a first step towards the adiabatic theory of ionization of atoms by intense laser pulses, here we consider the simplest one-dimensional zero-range potential model. The asymptotic solution to the time-dependent Schroedinger equation in the adiabatic regime is obtained and the photoelectron spectrum is calculated. The factorization formula for the photoelectron spectrum in the back-rescattering region, first suggested by Morishita et al. [Phys. Rev. Lett. 100, 013903 (2008)] on the basis of ab initio calculations, is derived analytically.

  12. Penning collisions of laser-cooled metastable helium atoms

    Science.gov (United States)

    Pereira Dos Santos, F.; Perales, F.; Léonard, J.; Sinatra, A.; Wang, Junmin; Saverio Pavone, F.; Rasel, E.; Unnikrishnan, C. S.; Leduc, M.

    2001-04-01

    We present experimental results on the two-body loss rates in a magneto-optical trap of metastable helium atoms. Absolute rates are measured in a systematic way for several laser detunings ranging from -5 to -30 MHz and at different intensities, by monitoring the decay of the trap fluorescence. The dependence of the two-body loss rate coefficient β on the excited state ( 23P2) and metastable state ( 23S1) populations is also investigated. From these results we infer a rather uniform rate constant Ksp = (1+/-0.4)×10-7 cm3/s.

  13. Atomic lifetime measurements by beam-gas-dye laser spectroscopy

    Science.gov (United States)

    Schmoranzer, H.; Volz, U.

    1993-01-01

    Beam-gas-dye laser spectroscopy as a precise, cascade-free and collision-free method for measuring atomic lifetimes and individual oscillator strengths is described. Its recent application to fine-structure levels of the KrI 5p configuration is reported. The experimental uncertainty is reduced by one order of magnitude, with respect to previous work, down to 0.3% (1σ). The discussion of these results in comparison with experimental and theoretical ones from the literature underlines the precision of the method and its potential to guide future theoretical developments.

  14. Approaches of output improvement for a cesium vapor laser pumped by a volume-Bragg-grating coupled laser-diode-array

    International Nuclear Information System (INIS)

    We report the approaches of output improvement for a cesium vapor laser, which was pumped by a volume-Bragg-grating (VBG) coupled broad-area laser-diode-array (LDA) with the quasi-continuous-wave (QCW) drive mode, in adopting an appropriate heating procedure and improving the pump configuration

  15. In-situ vaporization and matrix removal for the determination of rare earth impurities in zirconium dioxide by electrothermal vaporization inductively coupled plasma atomic emission spectrometry

    International Nuclear Information System (INIS)

    A novel method for the determination of trace rare earth impurities in ZrO2 powder has been developed based on electrothermal vaporization inductively coupled plasma atomic emission spectrometry. A polytetrafluoroethylene slurry was used as a fluorinating reagent to convert both the matrix (Zr) and the analytes (rare earth elements) into fluorides with different volatilities at a high temperature in a graphite furnace. The more volatile ZrF4 was removed in-situ by selective vaporization prior to the determination of the analytes, removing matrix spectral interferences. Under optimum operating conditions, the absolute detection limits of the analytes varied from 0.04 ng (Yb) to 0.50 ng (Pr) with relative standard deviations less than 5%. The recommended approach has been successfully applied to the determination of trace rare earth impurities (La, Pr, Eu, Gd, Ho and Yb) in ZrO2 powder and the results were in good agreement with those obtained by pneumatic nebulization inductively coupled plasma atomic emission spectrometry after the separation of the matrix using a solvent extraction procedure

  16. Energy absorption, ionization, and harmonic emission in laser-irradiated atomic clusters

    OpenAIRE

    Kundu, M.

    2007-01-01

    The excellent coupling of laser light to atomic clusters is a known, experimentally established fact. However, the physical mechanism of laser absorption is still controversially discussed. Linear resonance (LR) absorption occurs for sufficiently long laser pulses of optical or longer wavelengths. Here the Mie-plasma frequency initially rises above the laser frequency, then drops due to cluster expansion and therefore meets the laser frequency at some point. Instead, in few-cycle laser pulses...

  17. Coupling laser ablation and atomic fluorescence spectrophotometry: an example using mercury analysis of small sections of fish scales.

    Science.gov (United States)

    Beaudin, Luc; Johannessen, Sophia C; Macdonald, Robie W

    2010-11-01

    Mercury is a toxic element that exchanges among air, water, and sediments and biomagnifies into high trophic level organisms. Here, we present a novel combination of laser ablation with relatively low-cost cold vapor atomic fluorescence spectrophotometry to analyze Hg vaporized from targeted patches of fish scale 300-500 μm square. This method permits the analysis of multiple samples from the same scale, which is useful, because fish scale growth rings may provide an archive from which spatial and temporal trends in environmental Hg can be inferred at fine resolution. The detection limit of the method is 1.5 pg Hg, with a precision of 0.1 pg/μL. Developed using fish scales, the method could be adapted to other media, such as baleen, shells, nails, hair, teeth, wood and, possibly, varved sediments. PMID:20942426

  18. CO2 - LASER RADIATION ABSORPTION IN 1000 CM-1 WATER VAPOR CONTINUUM

    OpenAIRE

    Aref'Ev, V.; Sizov, N.; Dianov-Klokov, V.; V. Ivanov

    1980-01-01

    Water vapor absorption of CO2-laser radiation at R 40, R 10, P 20, P 32 lines of the 10.4µ band and R 10, R 18, R 44 lines of the 9.4µ band has been investigated in the laboratory. The results obtained are compared with the measurements of 10-13µ solar radiation attenuation. The experimental facts strongly support the assumption that water dimers play an important role in the 8-13µ region. The analysis of field and laboratory experiments allow the following conclusion : under most meteorologi...

  19. Fabrication of highly ultramicroporous carbon nanofoams by SF6-catalyzed laser-induced chemical vapor deposition

    Science.gov (United States)

    Hattori, Yoshiyuki; Shuhara, Ai; Kondo, Atsushi; Utsumi, Shigenori; Tanaka, Hideki; Ohba, Tomonori; Kanoh, Hirofumi; Takahashi, Kunimitsu; Vallejos-Burgos, Fernando; Kaneko, Katsumi

    2016-05-01

    We have developed a laser-induced chemical vapor deposition (LCVD) method for preparing nanocarbons with the aid of SF6. This method would offer advantages for the production of aggregates of nanoscale foams (nanofoams) at high rates. Pyrolysis of the as-grown nanofoams induced the high surface area (1120 m2 g-1) and significantly enhanced the adsorption of supercritical H2 (16.6 mg g-1 at 77 K and 0.1 MPa). We also showed that the pyrolized nanofoams have highly ultramicroporous structures. The pyrolized nanofoams would be superior to highly microporous nanocarbons for the adsorption of supercritical gases.

  20. Two-step resonance ionization spectroscopy of Na atomic beam using cw and pulsed lasers

    International Nuclear Information System (INIS)

    Two-step photoionization of sodium atomic beam has been carried out using a cw and a pulsed dye lasers. Sodium ions have been detected by a time of flight method in order to reduce background noise. With a proper power of the pulsed dye laser the sodium atomic beam has been irradiated by a resonant cw dye laser. The density of the sodium atomic beam is estimated to be 103 cm-3 at the ionization area. (author)

  1. Titanium atom detection by resonance fluorescence excited with a nitrogen laser

    International Nuclear Information System (INIS)

    Coincidence of wave lengths of nitrogen laser basing lines and resonance transitions in titanium atom is investigated. It is shown that resonance fluorescence excited by nitrogen laser can be used for absolute titanium atom density measurements. Experiments on titanium atom detection in a vapour cloud formed under irradiation of a titanium target in vacuum by dye laser pulse, are conducted. Fluorescence extinguishing is observed under high evaporation power

  2. QUANTUM STATISTICS OF AN ATOM LASER IN THEPRESENCE OF A STRONG INPUT LIGHT

    Institute of Scientific and Technical Information of China (English)

    JING HUI; MIAO YUAN-XIU; HAN YI-ANG

    2001-01-01

    Within the framework of quantum dynamical theory, we present a new method to control the quantum statistics of an atom laser by applying a powerful input light. Differing from the case in the rotating wave approximation, the non-classical properties can appear in the output atom laser beam with the evolution of time. By choosing a suitable phase of the input light, it is capable of realizing a steady and brighter output of coherent atom laser.

  3. Controlling quantum coherence of atom laser by light with strong strength

    Institute of Scientific and Technical Information of China (English)

    景辉; 葛墨林

    2002-01-01

    A new method for controlling the quantum coherence of atom laser by applying input light with strong strength is presented within the framework of quantum dynamical theory. Unlike the case of rotating wave approximation(RWA), we show that the non-classical properties, such as sub-Poisson distribution and quadrature squeezed effect, can appear in the output atom laser beam with time. By choosing suitable initial RF phase, a steady and brighter output of squeezed coherent atom laser is also available.

  4. Ionization of hydrogen atom by electron impact in the presence of elliptically polarized laser field

    International Nuclear Information System (INIS)

    The problem of ionization in electron hydrogen atom collision in the presence of elliptically polarized laser field, is investigated. The use of the higher order modification of the atomic bound state wave function shows that there is a strong enhancement in the cross section when the laser frequency is half the atomic transition frequency. The dependence of the cross section on the polarization of the laser field is also discussed. (author). 3 refs., 2 figs

  5. Hybrid lasers produced in potassium vapor by off-resonance pumping

    International Nuclear Information System (INIS)

    Pulsed amplified emissions are observed at or near atomic transitions cascading down from the K(6S) and K(4D5/2) states, when a pulsed dye laser is tuned near the K(6S left-arrow 43/2,1/2) and the K(4D5/2 left-arrow 4P3/2) transitions. Emissions are suppressed when the pulsed dye laser is tuned to the K(4D3/2 left-arrow 4P5/3,3/2) transitions. The pulsed dye laser is used to excite molecules in a heat-pipe oven from high-bring ro-vibrational levels in the K2(X1Σg+) ground state to ro-vibrational levels in the K2(B1 product u) state that predissociate to K(4S) and K(4P) atoms. The transitions can be pumped when the laser is tuned sufficiently close to the atomic resonances. We discuss the non-linear mechanisms responsible for the observed emissions. Emissions cascading down from the K(4S) state were first reported by Wang et al

  6. Simple analysis of total mercury and methylmercury in seafood using heating vaporization atomic absorption spectrometry.

    Science.gov (United States)

    Yoshimoto, Keisuke; Anh, Hoang Thi Van; Yamamoto, Atsushi; Koriyama, Chihaya; Ishibashi, Yasuhiro; Tabata, Masaaki; Nakano, Atsuhiro; Yamamoto, Megumi

    2016-01-01

    This study aimed to develop a simpler method for determining total mercury (T-Hg) and methylmercury (MeHg) in biological samples by using methyl isobutyl ketone (MIBK) in the degreasing step. The fat in the samples was extracted by MIBK to the upper phase. T-Hg transferred into the water phase. This was followed by the extraction of MeHg from the water phase using HBr, CuCl2 and toluene. The MeHg fraction was reverse-extracted into L-cysteine-sodium acetate solution from toluene. The concentrations of T-Hg and MeHg were determined by heating vaporization atomic absorption spectrometry. Certified reference materials for T-Hg and MeHg in hair and fish were accurately measured using this method. This method was then applied to determine T-Hg and MeHg concentrations in the muscle, liver and gonads of seafood for the risk assessment of MeHg exposure. The mean T-Hg and MeHg concentrations in squid eggs were 0.023 and 0.022 µg/g, and in squid nidamental glands 0.052 and 0.049 µg/g, respectively. The MeHg/T-Hg ratios in the eggs and nidamental glands of squid were 94.4% and 96.5%, respectively. The mean T-Hg and MeHg concentrations in the gonads of sea urchins were 0.043 and 0.001 µg/g, respectively, with a MeHg/T-Hg ratio of 3.5%. We developed an efficient analytical method for T-Hg and MeHg using MIBK in the degreasing step. The new information on MeHg concentration and MeHg/T-Hg ratios in the egg or nidamental glands of squid and gonads of sea urchin will also be useful for risk assessment of mercury in seafood. PMID:27432235

  7. Muonic atoms in super-intense laser fields

    Energy Technology Data Exchange (ETDEWEB)

    Shahbaz, Atif

    2009-01-28

    Nuclear effects in hydrogenlike muonic atoms exposed to intense high-frequency laser fields have been studied. Systems of low nuclear charge number are considered where a nonrelativistic description applies. By comparing the radiative response for different isotopes we demonstrate characteristic signatures of the finite nuclear mass, size and shape in the high-harmonic spectra. Cutoff energies in the MeV domain can be achieved, offering prospects for the generation of ultrashort coherent {gamma}-ray pulses. Also, the nucleus can be excited while the laser-driven muon moves periodically across it. The nuclear transition is caused by the time-dependent Coulomb field of the oscillating charge density of the bound muon. A closed-form analytical expression for electric multipole transitions is derived within a fully quantum mechanical approach and applied to various isotopes. The excitation probabilities are in general very small. We compare the process with other nuclear excitation mechanisms through coupling with atomic shells and discuss the prospects to observe it in experiment. (orig.)

  8. Comparison of electrothermal atomization diode laser Zeeman- and wavelength-modulated atomic absorption and coherent forward scattering spectrometry

    International Nuclear Information System (INIS)

    Atomic absorption and coherent forward scattering spectrometry by using a near-infrared diode laser with and without Zeeman and wavelength modulation were carried out with graphite furnace electrothermal atomization. Analytical curves and limits of detection were compared. The magnetic field was modulated with 50 Hz, and the wavelength of the diode laser with 10 kHz. Coherent forward scattering was measured with crossed and slightly uncrossed polarizers. The results show that the detection limits of atomic absorption spectrometry are roughly the same as those of coherent forward scattering spectrometry with crossed polarizers. According to the theory with bright flicker noise limited laser sources the detection limits and linear ranges obtained with coherent forward scattering spectrometry with slightly uncrossed polarizers are significantly better than those obtained with crossed polarizers and with atomic absorption spectrometry. This is due to the fact that employing approaches of polarization spectroscopy reduce laser intensity fluctuations to their signal carried fractions

  9. A compact and robust diode laser system for atom interferometry on a sounding rocket

    OpenAIRE

    Schkolnik, V.; Hellmig, O.; Wenzlawski, A.; Grosse, J.; Kohfeldt, A.; Döringshoff, K.; Wicht, A.; Windpassinger, P.; Sengstock, K.; Braxmaier, C.; Krutzik, M.; Peters, A

    2016-01-01

    We present a diode laser system optimized for laser cooling and atom interferometry with ultra-cold rubidium atoms aboard sounding rockets as an important milestone towards space-borne quantum sensors. Design, assembly and qualification of the system, combing micro-integrated distributed feedback (DFB) diode laser modules and free space optical bench technology is presented in the context of the MAIUS (Matter-wave Interferometry in Microgravity) mission. This laser system, with a volume of 21...

  10. A study on laser power balance in a multi-step ionization process of atoms

    International Nuclear Information System (INIS)

    Based on rate equation a theoretical study on laser power balance in a resonance multi-step ionization process of atoms has been presented in this paper. The calculation results made for a typical three-level atom show that there is an optimization laser power assignment when the total pumping laser power is limited, and under the optimization laser power assignment the ionization probability of a three-level atom can reach its maximum value. This conclusion is very different from that obtained under saturation excitation conditions. The method used here can be applied to more complicated multi-step ionization process of atoms. (authors)

  11. Laser physical and laser chemical vapor deposition of TiN and TiNxOy films

    International Nuclear Information System (INIS)

    The authors have investigated the formation of polycrystalline TiN and amorphous TiNxOy films using laser physical (LPVD) and laser chemical (LCVD) vapor deposition techniques. The LPVD method involved the ablation of a TiN hot pressed pellet and Ti in the presence of nitrogen plasma using nanosecond XeCl excimer laser pulses (wavelength 308nm, pulse duration 45 x 10-9 seconds, and energy density ∼ 4-5 Jcm-2). The films were polycrystalline (average grain size ∼ 100 angstrom) with face-centered-cubic structure and lattice constant of 4.25 angstrom. The average grain size remained constant as the substrate temperature ranged from 25 to 550 degrees C. In the LCVD method, a pulsed CO2 laser beam was used to crack TiCl4 and NH3 and from TiN films. Amorphous TiNxOy films were formed under poor vacuum conditions in the LPVD techniques. These amorphous TiNxOy films often exhibited explosive recrystallization with characteristic star patterns. Resistivity and microhardness measurements were made on these films and these results have been correlated with microstructure and chemical composition

  12. Vapor-air plum by explosion of nuclear power plant reactor at atomic submarine

    International Nuclear Information System (INIS)

    Scenario of hypothetic accident with nuclear submarine is given. Equations for calculating gas-dynamic, geometrical and concentrational characteristics of the formed short vapor-air plum are presented. Example for calculating vapor-air plum during hypothetic accident with nuclear submarine is given. 3 refs., 6 figs

  13. COMPARISON OF AIR POLLUTANT EMISSIONS FROM VAPORIZING AND AIR ATOMIZING WASTE OIL HEATERS

    Science.gov (United States)

    The paper gives results of a characterization of gaseous and particulate emissions and vaporizing pot solid residues resulting from the combustion of waste crankcase oil in space heaters. Two types of waste oil burners were tested: a vaporizing oil burner rated at 35.2 kW, and an...

  14. Laser chemical vapor deposition of W on Si and SiO2/Si

    International Nuclear Information System (INIS)

    Direct write of W on bare Si and native SiO2/Si substrates has been investigated in an laser chemical vapor deposition (LCVD) system. W deposits on bare Si surface via the Si and/or H2 reduction of WF6 were self-limited in thickness to 200 - 600 Angstrom in both cases. Auger electron spectroscopic analysis showed that Si-H bonds could be poisoning the further growth of W. W deposits on native SiO2/Si were only obtainable via the H2 reduction WF6 in our laser direct-write system. The authors' experimental kinetic study indicates that HF desorption from the surface is the rate-controlling step for W deposition via the H2 reduction WF6

  15. Polycystic ovarian disease treated by laparoscopic argon laser capsule drilling: comparison of vaporization versus perforation technique.

    Science.gov (United States)

    Heylen, S M; Puttemans, P J; Brosens, I A

    1994-06-01

    Forty-four anovulatory women with polycystic ovarian disease (PCOD) were laparoscopically treated with the argon laser. Eighty percent of them were previously resistant to clomiphene citrate therapy. After surgery spontaneous ovulation occurred in 80% of the women. Spontaneous conception occurred in 55% of patients, and another 18% of the women who were previously resistant to clomiphene citrate conceived post-operatively after clomiphene citrate therapy. This gives an overall conception rate of 73% after 18 months (using life table analysis). Two different drilling techniques were used: classical vaporization of the ovarian capsule (22 women), and simple perforation of the ovarian capsule with subcapsular destruction of the ovarian stroma (22 women). No different ovulation or pregnancy rates were observed post-operatively between the two techniques. These results suggest that patients with PCOD can be induced to ovulate, and subsequently conceive, by laparoscopic argon laser treatment. The technique with minimal trauma to the ovarian capsule seems preferable. PMID:7962372

  16. Fabrication of CdTe solar cells by laser-driven physical vapor deposition

    Energy Technology Data Exchange (ETDEWEB)

    Compaan, A.; Bhat, A.; Tabory, C.; Liu, S.; Nguyen, M.; Aydinli, A.; Tsien, L.H.; Bohn, R.G. (Toledo Univ., OH (USA). Dept. of Physics and Astronomy)

    1991-05-01

    Polycrystalline cadmium sulfide-cadmium telluride heterojunction solar cells were fabricated for the first time using a laser-driven physical vapor deposition method. An XeCl excimer laser was used to deposit both of the II-VI semiconductor layers in a single vacuum chamber from pressed powder targets. Results are presented from optical absorption. Raman scattering, X-ray diffraction, and electrical characterization of the films. Solar cells were fabricated by deposition onto SnO{sub 2}-coated glass with top contacts produced by gold evaporation. Device performance was evaluated from the spectral quantum efficiency and current-voltage measurements in the dark and with air mass 1.5 solar illumination. (orig.).

  17. Gas-dynamic acceleration of laser-ablation plumes: Hyperthermal particle energies under thermal vaporization

    Science.gov (United States)

    Morozov, A. A.; Evtushenko, A. B.; Bulgakov, A. V.

    2015-02-01

    The expansion of a plume produced by low-fluence laser ablation of graphite in vacuum is investigated experimentally and by direct Monte Carlo simulations in an attempt to explain hyperthermal particle energies for thermally vaporized materials. We demonstrate that the translation energy of neutral particles, ˜2 times higher than classical expectations, is due to two effects, hydrodynamic plume acceleration into the forward direction and kinetic selection of fast particles in the on-axis region. Both effects depend on the collision number within the plume and on the particles internal degrees of freedom. The simulations allow ablation properties to be evaluated, such as ablation rate and surface temperature, based on time-of-flight measurements. Available experimental data on kinetic energies of various laser-produced particles are well described by the presented model.

  18. Continuous-wave, single-frequency 229 nm laser source for laser cooling of cadmium atoms

    OpenAIRE

    Kaneda, Yushi; Yarborough, J. M.; Merzlyak, Yevgeny; Yamaguchi, Atsushi; Hayashida, Keitaro; Ohmae, Noriaki; Katori, Hidetoshi

    2016-01-01

    Continuous-wave output at 229 nm for the application of laser cooling of Cd atoms was generated by the 4th harmonic using two successive second harmonic generation stages. Employing a single-frequency optically pumped semiconductor laser as a fundamental source, 0.56 W of output at 229 nm was observed with a 10-mm long, Brewster-cut BBO crystal in an external cavity with 1.62 W of 458 nm input. Conversion efficiency from 458 nm to 229 nm was more than 34%. By applying a tapered amplifier as a...

  19. A Scheme of Generating and Spatially Separating Two-Component Entangled Atom Lasers

    OpenAIRE

    Liu, Xiong-Jun; Jing, Hui; Liu, Xin; Zhan, Ming-sheng; Ge, Mo-Lin

    2005-01-01

    Entanglement of remote atom lasers is obtained via quantum state transfer technique from lights to matter waves in a five-level $M$-type system. The considered atom-atom collisions can yield an effective Kerr susceptibility for this system and lead to the self- and cross- phase modulation between the two output atom lasers. This effect results in generation of entangled states of output fields. Particularly, under different conditions of space-dependent control fields, the entanglement of ato...

  20. Laser spectroscopy of atoms in superfluid helium for the measurement of nuclear spins and electromagnetic moments of radioactive atoms

    Energy Technology Data Exchange (ETDEWEB)

    Fujita, T., E-mail: tomomi.fujita@riken.jp [Osaka University, Department of Physics (Japan); Furukawa, T. [Tokyo Metropolitan University, Department of Physics (Japan); Imamura, K.; Yang, X. F. [RIKEN Nishina Center (Japan); Hatakeyama, A. [Tokyo University of Agriculture and Technology, Department of Applied Physics (Japan); Kobayashi, T. [RIKEN Center for Advanced Photonics (Japan); Ueno, H. [RIKEN Nishina Center (Japan); Asahi, K. [Tokyo Institute of Technology, Department of Physics (Japan); Shimoda, T. [Osaka University, Department of Physics (Japan); Matsuo, Y. [Hosei University, Department of Advanced Sciences (Japan); Collaboration: OROCHI Collaboration

    2015-11-15

    A new laser spectroscopic method named “OROCHI (Optical RI-atom Observation in Condensed Helium as Ion catcher)” has been developed for deriving the nuclear spins and electromagnetic moments of low-yield exotic nuclei. In this method, we observe atomic Zeeman and hyperfine structures using laser-radio-frequency/microwave double-resonance spectroscopy. In our previous works, double-resonance spectroscopy was performed successfully with laser-sputtered stable atoms including non-alkali Au atoms as well as alkali Rb and Cs atoms. Following these works, measurements with {sup 84−87}Rb energetic ion beams were carried out in the RIKEN projectile fragment separator (RIPS). In this paper, we report the present status of OROCHI and discuss its feasibility, especially for low-yield nuclei such as unstable Au isotopes.

  1. Laser spectroscopy of atoms in superfluid helium for the measurement of nuclear spins and electromagnetic moments of radioactive atoms

    International Nuclear Information System (INIS)

    A new laser spectroscopic method named “OROCHI (Optical RI-atom Observation in Condensed Helium as Ion catcher)” has been developed for deriving the nuclear spins and electromagnetic moments of low-yield exotic nuclei. In this method, we observe atomic Zeeman and hyperfine structures using laser-radio-frequency/microwave double-resonance spectroscopy. In our previous works, double-resonance spectroscopy was performed successfully with laser-sputtered stable atoms including non-alkali Au atoms as well as alkali Rb and Cs atoms. Following these works, measurements with 84−87Rb energetic ion beams were carried out in the RIKEN projectile fragment separator (RIPS). In this paper, we report the present status of OROCHI and discuss its feasibility, especially for low-yield nuclei such as unstable Au isotopes

  2. Study of the interaction of atoms with strong laser fields

    International Nuclear Information System (INIS)

    Three aspects of the interactions of atoms with high intensity laser fields were treated. All three were motivated by experiment. The first investigation was prompted by a recent experiment (Kruit et al. 1983) involving multiphoton ionization of Xe. In this experiment it was found that the photoelectron energy spectrum contained peaks that corresponded to the absorption of more than the minimum number of photons required to ionize the atom. A model approximation here showed good qualitative agreement with experiment. An experiment (Grove et al. 1977) designed to test a theoretical calculation of the dynamical Stark effect stimulated the second part of this thesis, namely: a study of how an adiabatically and near-adiabatically changing field intensity affects the resonance fluorescence spectrum of a two-level atom. It was found that there is an asymmetry in the spectrum for off-resonance excitation produced because the field turn-on repopulates the dressed state that is depopulated by spontaneous emission. The third part of this thesis was based on an experiment (Granneman and Van der Wiel 1976) that attempted to verify a perturbation calculation of the two-photon ionization cross section of Cs. A discrepancy of four orders of magnitude near a minimum in the cross section was found between theory and experiment. To explain this discrepancy it was suggested (Armstrong and Beers 1977) that the effective order of nonlinearity (k) for this process varied significantly around the minimum. This study involves a perturbation calculation of k. It was found that k varies rapidly around the minimum, and that this variation should be experimentally observable for laser intensities of the order of tens of GW cm-2

  3. High-temperature quadrupole mass spectrometer for studying vaporization from materials heated by a CO2 laser

    International Nuclear Information System (INIS)

    To evaluate the effectiveness of mass spectrometry techniques in studying vaporization from selected materials, we designed a mass spectrometer than can be used either with a continuous wave or pulsed laser heating system or with a conventional furnace heating system. Our experimental apparatus, the components of which are described in detail, consisted of a quadrupole mass spectrometer positioned in a crossed-beam configuration, controlling electronics, a data acquisition system, a vacuum system, a cryogenic collimation system, and a laser heating system. Results of mass spectral scans taken during laser pyrolysis of polymeric materials and laser vaporization of graphite were compatible with data reported in other studies. Results of mass spectral studies of laser-induced combustion in the Ti + C system are also presented

  4. Spectral properties of a thresholdless dressed-atom laser

    CERN Document Server

    Luo, Min; Ficek, Zbigniew

    2010-01-01

    We investigate spectral properties of the atomic fluorescence and the output field of the cavity-mode of a single-atom dressed-state laser in a photonic crystal. We pay a particular attention to the behavior of the spectra in the presence of the frequency dependent reservoir and search for signatures of the thresholdless lasing. Although the thresholdless behavior has been predicted by analyzing the photon statistics of the cavity field, we find that the threshold behavior still exists in the spectrum of the cavity field. We find that the structure of cavity field spectrum depends strongly on the strange of the pumping rate. For low pumping rates, the spectrum is not monochromatic, it is composed of a set of discrete lines reveling the discrete (quantum) structure of the combined dressed-atom plus the cavity field system. We find that for a certain value of the pumping rate, the multi-peak structure converts into a single very narrow line centered at the cavity field frequency. A physical explanation of the b...

  5. Some new trends in laser isotope separation in atomic vapours

    International Nuclear Information System (INIS)

    New approaches to the methods of laser isotope separation are considered and realised which substantially extend the possibilities of the methods. To narrow down an absorption line and decrease parasitic absorption at transitions in isotope atoms that do not belong to an isotope being separated, two-photon excitation of atoms was used both in collinear and counterpropagating light beams. By using two-photon excitation in counterpropagating light beams, the weight amounts of Zn isotopes were separated under the conditions when the isotopic structure of a resonance transition was completely masked by the Doppler broadening. Two-photon excitation in collinear beams was used for efficient purification of lead from a rare 210Pb isotope to obtain a low-radioactive lead. A detailed computer simulation of separation of isotopes of Zn, B, Pb, and Si using two-photon excitation was performed. An efficient method of isotope separation involving chemical reactions with selectively excited long-lived atoms was proposed and realised. The method offers some advantages over the conventional photoionisation method. (invited paper)

  6. Laser scattering diagnostics of an argon atmospheric-pressure plasma jet in contact with vaporized water

    Science.gov (United States)

    Seo, B. H.; Kim, J. H.; You, S. J.; Seong, D. J.

    2015-12-01

    The radial profiles of the electron density, electron temperature, and molecular rotational temperature are investigated in an argon atmospheric-pressure plasma jet in contact with vaporized water, which is driven by a 13.56 MHz radio frequency by means of the Thomson and Raman laser scattering methods. There is a distinct difference in the radial profiles of the plasma parameters between plasmas in contact with water and those without water contact. In the case of plasmas without vaporized water contact, all the parameters have a single-peak distribution with maximum values at the center of the discharge. In the case of plasmas in contact with vaporized water, all parameters have double-peak distributions; a neighboring peak appears beside the main peak. The new peak may have originated from the ripple of the water surface, which works as a cathode, and the peak of the ripple offers a sharp curvature point, playing the role of a pin. Our experimental results and the underlying physics are described in detail.

  7. Two Types of Mass Abundance Distributions for Anionic Carbon Clusters Investigated by Laser Vaporization and Pulsed Molecular Beam Techniques

    Institute of Scientific and Technical Information of China (English)

    ZHAI Hua-Jin; LIU Bing-Chen; NI Guo-Quan; XUZhi-Zhan

    2000-01-01

    Two types of mass spectra for anionic carbon clusters Cn- have been revealed using laser vaporization and pulsed molecular beam techniques. The less structured mass spectrum characteristic of the magic-numbers at n = 5, 8,11, 15, and 17 is established at the early stage of the cluster formation process, namely, in the laser vaporization process. The more structured one is featured for a regular odd-even alternation and the magic numbers at n =10, 12, 16, 18, 22, and 28, and has been developed only after extensive clustering and qnenching processes, where low-energy electron attachment plays a vital role. Transition between these two types of mass spectra can be realized by controlling either the strength of the pulsed gas flow or the synchronism between the gas flow and the laser vaporization.

  8. Confinement of ultracold atoms in a Laguerre-Gaussian laser beam created with diffractive optics

    CERN Document Server

    Kennedy, Sharon A; Farrar, J Tom; Akin, T G; Krzyzewski, S; Abraham, E R I

    2013-01-01

    We report 2D confinement of Rb 87 atoms in a Laguerre-Gaussian laser beam. Changing of the sign of the detuning from the atomic resonance dramatically alters the geometry of the confinement. With the laser detuned to the blue, the atoms are confined to the dark, central node of the Laguerre-Gaussian laser mode. This trapping method leads to low ac Stark shifts to the atomic levels. Alternatively, by detuning the laser to the red of the resonance, we confine atoms to the high intensity outer ring in a multiply-connected, toroidal configuration. We model the confined atoms to determine azimuthal intensity variations of the trapping laser, caused by slight misalignments of the Laguerre-Gaussian mode generating optics.

  9. Behavior of vapor/plasma within the keyhole and above the workpiece during CO2 laser penetration welding

    Institute of Scientific and Technical Information of China (English)

    2008-01-01

    In this paper, a high-speed camera and an optical emission monitor were used to study the behavior of vapor/plasma during CO2 laser welding of SUS304 stainless steel. Results of optical emission from vapor/plasma show that two characteristic frequency bands exist, 100-500 Hz and 1 500-3 500 Hz. At the same time, the changing images of vapor/plasma and bottom pool also confirm that there are two different fluctuation frequency bands. One of the frequency bands represents the characteristic of vapor/plasma within the keyhole, and it is within 167-500 Hz. Another frequency band is within 1 500-3 500 Hz, and it obviously derives from the shielding gas. Some factors may cause these frequency differences between the keyhole plasma and the shielding gas plasma. One of them is that the vapor/plasma pressure within the keyhole will increase slowly.

  10. Multiphoton ionization of the hydrogen atom exposed to circularly or linearly polarized laser pulses

    International Nuclear Information System (INIS)

    This paper studies the multiphoton ionization of the hydrogen atom exposed to the linearly or circularly polarized laser pulses by solving the time-dependent Schrödinger equation. It finds that the ratio of the ionization probabilities by linearly and circularly polarized laser pulses varies with the numbers of absorbing photons. With the same laser intensity, the circularly polarized laser pulse favors to ionize the atom with more ease than the linearly polarized laser pulse if only two or three photons are necessary to be absorbed. For the higher order multiphoton ionization, the linearly polarized laser pulse has the advantage over circularly polarized laser pulse to ionize the atom. (atomic and molecular physics)

  11. All-atom force field for the prediction of vapor-liquid equilibria and interfacial properties of HFA134a.

    Science.gov (United States)

    Peguin, Robson P S; Kamath, Ganesh; Potoff, Jeffrey J; da Rocha, Sandro R P

    2009-01-01

    A new all-atom force field capable of accurately predicting the bulk and interfacial properties of 1,1,1,2-tetrafluoroethane (HFA134a) is reported. Parameterization of several force fields with different initial charge configurations from ab initio calculations was performed using the histogram reweighting method and Monte Carlo simulations in the grand canonical ensemble. The 12-6 Lennard-Jones well depth and diameter for the different HFA134a models were determined by fitting the simulation results to pure-component vapor-equilibrium data. Initial screening of the force fields was achieved by comparing the calculated and experimental bulk properties. The surface tension of pure HFA134a served as an additional screening property to help discriminate an optimum model. The proposed model reproduces the experimental saturated liquid and vapor densities, and the vapor pressure for HFA134a within average errors of 0.7%, 4.4%, and 3.1%, respectively. Critical density, temperature, vapor pressure, normal boiling point, and heat of vaporization at 298 K are also in good agreement with experimental data with errors of 0.2%, 0.1%, 6.2%, 0%, 2.2%, respectively. The calculated surface tension is found to be within the experimental range of 7.7-8.1 mN.m(-1). The dipole moment of the different models was found to significantly affect the prediction of the vapor pressure and surface tension. The ability of the HFA134a models in predicting the interfacial tension against water is also discussed. The results presented here are relevant in the development of technologies where the more environmentally friendly HFA134a is utilized as a substitute to the ozone depleting chlorofluorocarbon propellants. PMID:19086791

  12. Design, fabrication and characterization of tunable external cavity diode laser and atom trapping chips for atomic physics

    Science.gov (United States)

    Chuang, Ho-Chiao

    External cavity diode laser systems (ECDLs) have been well documented for their suitability in the fields of laser cooling and atom trapping, and are now widely used in optical and atomic physics. A particularly simple implementation of this idea uses feedback from a diffraction grating mounted in the Littrow configuration and the typical size of this laser is quite large (120mmx90mmx90mm). For atom optics, the current atom trapping chips are not in a feedthrough configuration, which makes the chips to glass cell assembly process complicated and the wires and solder areas vulnerable, resulting in an unreliable vacuum seal. Recent experimental realizations of atom optical devices such as atomic waveguides, beam splitters, and on-chip Bose-Einstein condensate (BEC) sources have opened a new field for the development of more complex devices such as, e.g., BEC-based atom transistor. This work focuses on micro/nano fabrication techniques to build three different devices for the miniature BEC system. The research work focuses on the development of new ECDLs, a novel fabrication process of feedthrough atom trapping chips for atomic optics and a fabrication process for atom transistor chips. In the ECDLs part, we describe a new method for constructing a smaller external-cavity diode laser by use of a micromachined silicon flexure and a VHG (Volume Holographic Grating). It is much smaller, inexpensive and easy to build because it is based on simple modifications of a few commercial optical and mechanical components but with a specific silicon flexure design enabled by micro-fabrication technology for the laser frequency tuning. In the feedthrough chips part, we present a novel fabrication process for feedthrough atom trapping chips in atomic condensate optics cells using the copper electroplating to seal the vias. The advantages of using feedthrough atom trapping chips are the simple microfabrication process and reduction of the overall chip area bonded on the glass atom

  13. Role of fluorine atoms in the oxidation-hydrolysis process of plasma assisted chemical vapor deposition fluorinated silicon nitride film

    Energy Technology Data Exchange (ETDEWEB)

    Sanchez, O.; Gomez-Aleixandre, C.; Palacio, C. (Universidad Autonoma de Madrid (Spain))

    The oxidation and/or hydrolysis of a plasma assisted chemical vapor deposition fluorinated silicon nitride film in a moisture atmosphere has been studied. The film presents fluorine atoms incorporated as -SiF, -SiF[sub 2], -SiF[sub 3], and [-SiF[sub 2]-][sub n] groups. The open structure of the film, due to the high fluorine content as [-SiF[sub 2]-][sub n], favors the penetration of oxygen and water molecules in the network. The evolution of the film has been explained by the different reactivity of the silicon atoms depending on their chemical environment. The role of fluorine atoms incorporated into the film has been established. 12 refs., 3 figs., 1 tab.

  14. Relativistic theory of atom-laser interactions at very high laser intensities

    International Nuclear Information System (INIS)

    The high-frequency approximation of Kristic and Mittleman is considered in detail as a basis for the relativistic theory of the atom-laser interactions. The properties of the 3D potentials are discussed. Within a one-dimensional model, similar to that employed by Kylstra, Ermolaev, and Joachain in ab initio calculations on the time-dependent Dirac equation, the electron mass-shift due to dressing by a superstrong laser field is investigated. In the full domain of the laser parameters, frequency ω and the peak field strength Ε0, the 1D bound states exhibit remarkable features. The numerical calculations show the existence of a very wide intermediate range of the field strengths where, in the zeroth-order of the high-frequency approximation, the binding is stabilized by the field

  15. A high-power laser transmitter for ground-based and airborne water-vapor measurements in the troposphere

    OpenAIRE

    Schiller, Max

    2009-01-01

    A gain-switched high-power single-frequency Ti:sapphire laser was developed. It is pumped with a frequency-doubled diode-pumped Nd:YAG laser. The laser fulfills the requirements for a transmitter of a water-vapor differential absorption lidar (DIAL), intended for accurate high temporally- and spatially-resolved measurements from the ground to the upper troposphere. The laser was developed using thermal, resonator-design, spectral, and pulse-evolution models. There were layouts assembled for o...

  16. Specializing and upgrading (single bunch) of AR and atomic physics: photo excitation/ionization of laser exciting atom, TOF measurement of photoion and photoelectron, etc

    International Nuclear Information System (INIS)

    By RF 2.5 GeV ring, many active measurements such as photoexcitation and photoionization of atom, photoion and adsorption of rare gas, photoelectron of metal vapor were investigated. Then, TOF measurement of photoion and photoionization of ion have been studied and good results were obtained. But the experiments of atom and molecule have not been observed by AR ring, because that many works of atomic physics were studied by the vacuum ultraviolet and soft x-ray field, and RF was easy to use. With specializing and upgrading of Ar, we discussed the atomic physical experiment using AR. By laser ablation, odd parity and even parity resonance of Li and the change of oscillator strength distribution of Ba were observed. Many problems were proposed on TOF measurement of photoion such as escape of the light element, recombination of multiion, thermal ion and the ratio of pulse width/period. To solve these problems, the electron start-ion stop method and the photon start-ion stop method were suggested. TOF measurement of photoelectron has features such as (1) the simultaneous measurement of the wide range of energy, (2) good character in the low energy field and (3) constant background. (S.Y.)

  17. Nanoscale focused ion beam from laser-cooled lithium atoms

    International Nuclear Information System (INIS)

    We demonstrate a new type of nanoscale focused ion beam (FIB) based on photoionizing laser-cooled atoms held at millikelvin temperatures in a magneto-optical trap (MOT). This new source expands the range of available ionic species and accessible ion beam energies for FIBs, enhancing their role as one of the most important tools for nanoscale characterization and fabrication. We show examples of microscopy with lithium ions obtained by scanning the FIB and collecting the resulting secondary electrons, and characterize the beam focus by a 25-75% rise distance measurement of (26.7 ± 1.0) nm at a beam energy of 2 keV. We also examine the dependence of the focal size on MOT temperature and beam energy. (paper)

  18. Creation of an Ultracold Plasma by Photoionizing Laser-Cooled Cesium Atom

    Institute of Scientific and Technical Information of China (English)

    JING Qun; FENG Zhi-Gang; ZHANG Lin-Jie; LI Chang-Yong; ZHAO Jian-Ming; JIA Suo-Tang

    2008-01-01

    @@ The signals of ultracold plasma are observed by two-photon ionization of laser-cooled atom in a caesium magneto-optical trap.A simple model has been introduced to explain the creation of plasma, and the mechanism is further investigated by changing the energy of a pulsed dye laser and the number of initial cooled atoms.

  19. Request for Support for the Conference on Super Intense Laser Atom Physics

    International Nuclear Information System (INIS)

    The Conference on Super Intense Laser Atom Physics (SILAP) was held in November 2003 in Dallas, Texas. The venue for the meeting was South Fork Ranch in the outskirts of Dallas. The topics of the meeting included high harmonic generation and attosecond pulse generation, strong field interactions with molecules and clusters, particle acceleration, and relativistic laser atom interactions

  20. SOME PROPERTIES OF ATOMIC BEAM PRODUCED BY LASER INDUCED ABLATION OF Li TARGET

    OpenAIRE

    Harnafi, M.; Dubreuil, B.

    1987-01-01

    In this experiment, pulsed atomic beams produced in vacuum by laser induced ablation from lithium target are analyzed by laser-induced fluorescsence (LIF). As an application of this atomic beam production technique, the l-mixing processes induced in the n = 9, 10 Li Rydberg states by collisions with CO2 molecules have been investigated.

  1. Flow injection-chemical vapor generation atomic fluorescence spectrometry hyphenated system for organic mercury determination: A step forward

    Energy Technology Data Exchange (ETDEWEB)

    Angeli, Valeria [National Research Council of Italy, C.N.R., Istituto di Chimica dei Composti Organo Metallici - ICCOM-UOS Pisa, Area di Ricerca, Via G. Moruzzi 1, 56124 Pisa (Italy); Biagi, Simona [National Research Council of Italy, C.N.R., Istituto per i Processi Chimico-Fisici - IPCF-UOS Pisa, Area di Ricerca, Via G. Moruzzi 1, 56124 Pisa (Italy); Ghimenti, Silvia [University of Pisa, Department of Chemistry and Industrial Chemistry, Via Risorgimento 35, 56126 Pisa (Italy); Onor, Massimo; D' Ulivo, Alessandro [National Research Council of Italy, C.N.R., Istituto di Chimica dei Composti Organo Metallici - ICCOM-UOS Pisa, Area di Ricerca, Via G. Moruzzi 1, 56124 Pisa (Italy); Bramanti, Emilia, E-mail: bramanti@pi.iccom.cnr.it [National Research Council of Italy, C.N.R., Istituto di Chimica dei Composti Organo Metallici - ICCOM-UOS Pisa, Area di Ricerca, Via G. Moruzzi 1, 56124 Pisa (Italy)

    2011-11-15

    Monomethylmercury and ethylmercury were determined on line using flow injection-chemical vapor generation atomic fluorescence spectrometry without neither requiring a pre-treatment with chemical oxidants, nor UV/MW additional post column interface, nor organic solvents, nor complexing agents, such as cysteine. Inorganic mercury, monomethylmercury and ethylmercury were detected by atomic fluorescence spectrometry in an Ar/H{sub 2} miniaturized flame after sodium borohydride reduction to Hg{sup 0}, monomethylmercury hydride and ethylmercury hydride, respectively. The effect of mercury complexing agent such as cysteine, ethylendiaminotetracetic acid and HCl with respect to water and Ar/H{sub 2} microflame was investigated. The behavior of inorganic mercury, monomethylmercury and ethylmercury and their cysteine-complexes was also studied by continuous flow-chemical vapor generation atomic fluorescence spectrometry in order to characterize the reduction reaction with tetrahydroborate. When complexed with cysteine, inorganic mercury, monomethylmercury and ethylmercury cannot be separately quantified varying tetrahydroborate concentration due to a lack of selectivity, and their speciation requires a pre-separation stage (e.g. a chromatographic separation). If not complexed with cysteine, monomethylmercury and ethylmercury cannot be separated, as well, but their sum can be quantified separately with respect to inorganic mercury choosing a suitable concentration of tetrahydroborate (e.g. 10{sup -5} mol L{sup -1}), thus allowing the organic/inorganic mercury speciation. The detection limits of the flow injection-chemical vapor generation atomic fluorescence spectrometry method were about 45 nmol L{sup -1} (as mercury) for all the species considered, a relative standard deviation ranging between 1.8 and 2.9% and a linear dynamic range between 0.1 and 5 {mu}mol L{sup -1} were obtained. Recoveries of monomethylmercury and ethylmercury with respect to inorganic mercury were

  2. Efficient multiple time scale method for modeling compressible vapor plume dynamics inside transient keyhole during fiber laser welding

    Science.gov (United States)

    Pang, Shengyong; Chen, Xin; Li, Wen; Shao, Xinyu; Gong, Shuili

    2016-03-01

    Efficient coupling modeling of multiple time scale interactions between keyhole, weld pool and compressible vapor plume during laser welding has long been limited. To address this problem, we present a highly efficient multiple time scale method combining a novel dual-time stepping and Ghost Fluid interpolation strategy with incompressible and compressible fluid solvers, which allows us predicting the compressible plume dynamics inside transient keyhole in fiber laser welding for the first time. In our method, the compressible dynamic vapor inside the transient keyhole is solved with a Roe scheme based algorithm and the incompressible molten liquid of weld pool is calculated by a Projection method. A novel temperature dependent boundary condition of vapor plume is also proposed for the consideration of the dynamic evaporation phenomena on the transient keyhole wall. It is found that the time dependent distributions of vapor plume characteristics, including temperature, pressure, velocity, density and Mach number distributions inside the transient keyhole induced by laser welding can be reasonably predicted by comparing to experimental and literature data. It is also shown that the proposed multiple time scale method is around 60 times faster than the vapor plume modeling method using a single nanosecond scale time step. For the vapor plume in a typical fiber laser welding process, the results indicate that the peak pressure can be greater than 2.0 atmospheric pressures; the average density is around 0.15-0.3 kg/m3 which is much smaller than the air density; and the local Mach number can be greater than 0.8 or even 1.0 Mach which demonstrates the necessity to treat the vapor plume as a compressible fluid.

  3. Dynamic characteristics and mechanisms of compressible metallic vapor plume behaviors in transient keyhole during deep penetration fiber laser welding

    Science.gov (United States)

    Pang, Shengyong; Shao, Xinyu; Li, Wen; Chen, Xin; Gong, Shuili

    2016-07-01

    The compressible metallic vapor plume or plasma plume behaviors in the keyhole during deep penetration laser welding have significant effects on the joint quality. However, these behaviors and their responses to process parameter variations have not been well understood. In this paper, we first systematically study the dynamic characteristics and mechanisms of compressible metallic vapor plume behaviors in transient keyhole during fiber laser welding of 304 stainless steels based on a multiple timescale multiphase model. The time-dependent temperature, pressure, velocity and Mach number distributions of vapor plume under different process parameters are theoretically predicted. It is found that the distributions of the main physical characteristics of vapor plume such as pressure, velocity as well as Mach number in keyhole are usually highly uneven and highly time dependent. The peak difference of the velocity, pressure, temperature and Mach number of the vapor plume in a keyhole could be greater than 200 m/s, 20 kPa, 1000 K and 0.6 Mach, respectively. The vapor plume characteristics in a transient keyhole can experience significant changes within several hundreds of nanoseconds. The formation mechanisms of these dynamic characteristics are mainly due to the mesoscale keyhole hump (sized in several tens of microns) dynamics. It is also demonstrated that it is possible to suppress the oscillations of compressible vapor plume in the keyhole by improving the keyhole stability through decreasing the heat input. However, stabilizing the keyhole could only weaken, but not eliminate, the observed highly uneven and transient characteristics. This finding may pose new challenges for accurate experimental measurements of vapor plume induced by laser welding.

  4. Stationary entanglement between two spatially separated atoms driven by a coherent laser field

    Institute of Scientific and Technical Information of China (English)

    Liao Xiang-Ping; Fang Mao-Fa; Zheng Xiao-Juan; Cai Jian-Wu

    2007-01-01

    This paper studies quantum entanglement between two spatially separated atoms driven by a coherent laser field in the dissipative process of spontaneous emission. It is shown that the entanglement strongly depends on the detuning of the laser frequency from atomic transition frequency, the interatomic separation and the Rabi frequency of the coherent laser field. A considerable amount of steady state entanglement can be obtained near △ = -α(i.e., the dipole-dipole interaction and the detuning cancel out mutually) for small atomic separation and large Rabi frequency of the coherent laser field.

  5. Determination of mercury in gasoline by cold vapor atomic absorption spectrometry with direct reduction in microemulsion media

    Science.gov (United States)

    Brandão, Geisamanda Pedrini; de Campos, Reinaldo Calixto; Luna, Aderval Severino

    2005-06-01

    The determination of Hg in gasoline by cold vapor atomic absorption spectrometry, after direct aqueous NaBH 4 reduction in a three-component (microemulsion) medium, was investigated. Microemulsions were prepared by mixing gasoline with propan-1-ol and 50% v / v HNO 3 at a 20 : 15 : 1 volume ratio. A long-term homogeneous system was immediately formed this way. After reduction, the Hg vapor generated in a reaction flask was transported to an intermediate K 2Cr 2O 7/H 2SO 4 trap solution in order to avoid poisoning of the Au-Pt trap by the gasoline vapors. A second reduction step was then conducted and the generated Hg vapor transported to the Au-Pt trap, followed by thermal release of Hg 0 and atomic absorption measurement. Purified N 2 was used as purge and transport gas. After multivariate optimization by central composite design calibration graphs showed coefficients of correlation of 0.9999 and a characteristic mass of 2 ng was obtained. Typical coefficients of variation of 5% and 6% were found for ten consecutive measurements at concentration levels of 1 and 8 μg L -1 of Hg 2+, respectively. The limit of detection was 0.10 μg L -1 (0.14 μg kg -1) in the original sample. A total measurement cycle took 11 min, permitting duplicate analysis of 3 samples per hour. The results obtained with the proposed procedure in the analysis of commercial gasoline samples were in agreement with those obtained by a comparative procedure. Gasoline samples of the Rio de Janeiro city have shown Hg concentrations below 0.27 μg L -1.

  6. Determination of mercury in gasoline by cold vapor atomic absorption spectrometry with direct reduction in microemulsion media

    International Nuclear Information System (INIS)

    The determination of Hg in gasoline by cold vapor atomic absorption spectrometry, after direct aqueous NaBH4 reduction in a three-component (microemulsion) medium, was investigated. Microemulsions were prepared by mixing gasoline with propan-1-ol and 50% v / v HNO3 at a 20 : 15 : 1 volume ratio. A long-term homogeneous system was immediately formed this way. After reduction, the Hg vapor generated in a reaction flask was transported to an intermediate K2Cr2O7/H2SO4 trap solution in order to avoid poisoning of the Au-Pt trap by the gasoline vapors. A second reduction step was then conducted and the generated Hg vapor transported to the Au-Pt trap, followed by thermal release of Hg0 and atomic absorption measurement. Purified N2 was used as purge and transport gas. After multivariate optimization by central composite design calibration graphs showed coefficients of correlation of 0.9999 and a characteristic mass of 2 ng was obtained. Typical coefficients of variation of 5% and 6% were found for ten consecutive measurements at concentration levels of 1 and 8 μg L-1 of Hg2+, respectively. The limit of detection was 0.10 μg L-1 (0.14 μg kg-1) in the original sample. A total measurement cycle took 11 min, permitting duplicate analysis of 3 samples per hour. The results obtained with the proposed procedure in the analysis of commercial gasoline samples were in agreement with those obtained by a comparative procedure. Gasoline samples of the Rio de Janeiro city have shown Hg concentrations below 0.27 μg L-1

  7. Mid-IR laser absorption diagnostics for hydrocarbon vapor sensing in harsh environments

    Science.gov (United States)

    Klingbeil, Adam Edgar

    unburned fuel, engine performance can be characterized and future engine designs can be improved to utilize all of the fuel supplied to the engine. Simultaneous measurement of absorption at two wavelengths is used as a basis for hydrocarbon detection in severe environments. A novel wavelength-tunable mid-IR laser is modified to rapidly switch between two wavelengths, improving the versatility of this laser system. The two-wavelength technique is then exploited to measure vapor concentration while rejecting interferences such as scattering from liquid droplets and absorption from other species. This two-wavelength laser is also used to simultaneously determine temperature and vapor concentration. These techniques, in combination with the library of temperature-dependent hydrocarbon spectra, lay the groundwork necessary to develop fuel diagnostics for laboratory experiments and tests in pulse detonation engines and internal combustion engines. The temperature-dependent spectroscopy of gasoline is examined to develop a sensor for fuel/air ratio in an internal combustion engine. A wavelength was selected for good sensitivity to gasoline concentration. A spectroscopic model is developed that uses the relative concentrations of five structural classes to predict the absorption spectrum of gasoline samples with varying composition. The model is tested on 21 samples of gasoline for temperatures ranging from 300 to 1200 K, showing good agreement between model and measurements over the entire temperature range. Finally, a two-wavelength diagnostic was developed to measure the post-evaporation temperature and n-dodecane concentration in an aerosol-laden shock tube. The experimental data validate a model which calculates the effects of shock-wave compression on a two-phase mixture. The measured post-shock temperature and vapor concentration compare favorably for gas-phase and aerosol experiments. The agreement between the two fuel-loading techniques verifies that this aerosol shock

  8. Time-resolved and doppler-reduced laser spectroscopy on atoms

    International Nuclear Information System (INIS)

    Radiative lifetimes have been studied in neutral boron, carbon, silicon and strontium, in singly ionized gadolinium and tantalum and in molecular carbon monoxide and C2. The time-resolved techniques were based either on pulsed lasers or pulse-modulated CW lasers. Several techniques have been utilized for the production of free atoms and ions such as evaporation into an atomic beam, sputtering in hollow cathodes and laser-produced plasmas. Hyperfine interactions in boron, copper and strontium have been examined using quantum beat spectroscopy, saturation spectroscopy and collimated atomic beam spectroscopy. Measurement techniques based on effusive hollow cathodes as well as laser produced plasmas in atomic physics have been developed. Investigations on laser produced plasmas using two colour beam deflection tomography for determination of electron densities have been performed. Finally, new possibilities for view-time-expansion in light-in-flight holography using mode-locked CW lasers have been demonstrated. (au)

  9. Explosive vaporization induced by high-power CO2-laser target interactions

    International Nuclear Information System (INIS)

    The interactions of high-power laser pulses with targets such as metals or dielectric materials causes a series of optical, thermal, and mechanical processes. Thereby, heating, melting, and vaporization can take place in a short time. At power densities of about 107 to several 108 W/cm2 this can even be produced explosively. As compared to continuous ablation, this type of interaction can remove greater masses from the bulk of material. The investigations are performed by using an electron-beam preionized CO2-laser acting on different target materials. The energy of the laser pulses is about 30 J, the pulse-half-widths of the long-tail pulses 4 to 6 μs. Optical measurements yield some information on threshold values for these processes, for the formation and expansion of plasmas, and for the ejection of material in form of greater particles. High speed photographic techniques include a rotating mirror- and an image converter camera. Starting from shock-wave theory, gas dynamic equations (in unidimensional approximation) allow for a quantitative determination of the specific internal energies and pressures in the case of optical detonation. (orig.)

  10. Laser Programs Highlights 1998

    Energy Technology Data Exchange (ETDEWEB)

    Lowdermilk, H.; Cassady, C.

    1999-12-01

    This report covers the following topics: Commentary; Laser Programs; Inertial Confinement Fusion/National Ignition Facility (ICF/NIF); Atomic Vapor Laser Isotope Separation (AVLIS); Laser Science and Technology (LS&T); Information Science and Technology Program (IS&T); Strategic Materials Applications Program (SMAP); Medical Technology Program (MTP) and Awards.

  11. Attoclock reveals natural coordinates of the laser-induced tunnelling current flow in atoms

    DEFF Research Database (Denmark)

    Pfeiffer, Adrian N.; Cirelli, Claudio; Smolarski, Mathias; Dimitrovski, Darko; Abu-Samha, Mahmoud; Madsen, Lars Bojer; Keller, Ursula

    2012-01-01

    In the research area of strong-laser-field interactions and attosecond science1, tunnelling of an electron through the barrier formed by the electric field of the laser and the atomic potential is typically assumed to be the initial key process that triggers subsequent dynamics1, 2, 3. Here we use...... for laser tunnel ionization in all atoms and in particular in larger molecular systems with correspondingly larger dipoles and polarizabilities....

  12. Ionization of hydrogen atom by X-ray absorption in the presence of optical laser field

    International Nuclear Information System (INIS)

    The absorption of X-rays in hydrogen atom considering the irradiation of the target by an intense optical laser of frequency ω is studied. It is found that the terms of the modified scattering amplitude has different dependence on polarization vectors of X-ray fields and laser fields. There is resonance in the differential cross section for absorption at different frequencies when ω (the laser frequency) becomes nearly equal to atomic transition frequency. (author). 21 refs., 2 figs

  13. Electron structure of atoms in laser plasma: The Debye shielding model

    International Nuclear Information System (INIS)

    The electronic structure and the energy spectra of multielectron atoms in laser plasmas are examined by the Debye shielding model. The effect of the plasma environment on the electrons bound in an atom is taken into account by introducing the screened Coulomb-type potentials into the electronic Hamiltonian of an atom in place of the standard nuclear attraction and electron repulsion potentials. The capabilities of this new Hamiltonian are demonstrated for He and Li in laser plasmas. (author)

  14. Development of long life pulse power supply for copper vapor laser. Do joki laser yo chojumyo reiki dengen no kaihatsu. ; Saidai shutsuryoku unten oyobi laser hasshin

    Energy Technology Data Exchange (ETDEWEB)

    Fujii, T.; Goto, N.; Nemoto, K. (Central Research Inst. of Electric Power Industry, Tokyo (Japan))

    1990-04-01

    Long life pulse power supply for Cu vapor laser was developed. This is composed of the pulse generation circuit and the pulse compression circuit. Current pulse of 10 mu second pulse width is generated in the pulse generating circuit by switching electric charge on the condensor charged through GTO (gate turn off) thyristors. The pulse compression circuit makes the current pulse fast to 300ms utilizing the difference of inductance at the saturation and the unsaturation on the circuit which uses a reactor having saturable property using a ferromagnetic substance for the core as the magnetic switch. The operation was carried out at the GTO generasting full power. Co base amorphous alloy of low loss was used for the core of saturable inductor and the circuit efficiency of 77% could be obtained by suppressing the heat generation in core even at 4,000Hz operation. The full output power of 8.2kW was possible which corresponds to 100W class laser oscillation. Repeated Cu vapor laser oscillation of 30W succeeded at the condition of 4,000Hz and power supply output of 5.9kW. 7 refs., 21 figs., 8 tabs.

  15. Determination of Hg(II) as a pollutant in Karachi coastal waters by cold vapor atomic absorption spectroscopy

    International Nuclear Information System (INIS)

    Now a days, environmental monitoring has great importance and mercury is well known for its toxicity. Mercury (which is at trace level) is analyzed by cold vapor atomic absorption spectroscopy with amendments that are appropriate to the present laboratory need. The results are consistent with previous analysis, through other methods, two areas namely Ibrahim Hyderi and Fisheries were found to have mercury levels around 0.193 mu/L and 0.110 mu g/L, respectively. Whereas other areas have mercury levels similar to other places reported earlier. (author)

  16. Organometallic chemical vapor deposition of silicon nitride films enhanced by atomic nitrogen generated from surface-wave plasma

    International Nuclear Information System (INIS)

    Organometallic chemical vapor deposition of silicon nitride films enhanced by atomic nitrogen generated from surface-wave plasma is investigated. Feasibility of precursors of triethylsilane (TES) and bis(dimethylamino)dimethylsilane (BDMADMS) is discussed based on a calculation of bond energies by computer simulation. Refractive indices of 1.81 and 1.71 are obtained for deposited films with TES and BDMADMS, respectively. X-ray photoelectron spectroscopy (XPS) analysis of the deposited film revealed that TES-based film coincides with the stoichiometric thermal silicon nitride

  17. Diode-laser-based water vapor differential absorption lidar (DIAL) profiler evaluation

    Science.gov (United States)

    Spuler, S.; Weckwerth, T.; Repasky, K. S.; Nehrir, A. R.; Carbone, R.

    2012-12-01

    We are in the process of evaluating the performance of an eye-safe, low-cost, diode-laser-based, water vapor differential absorption lidar (DIAL) profiler. This class of instrument may be capable of providing continuous water vapor and aerosol backscatter profiles at high vertical resolution in the atmospheric boundary layer (ABL) for periods of months to years. The technology potentially fills a national long term observing facility gap and could greatly benefit micro- and meso-meteorology, water cycle, carbon cycle and, more generally, biosphere-hydrosphere-atmosphere interaction research at both weather and climate variability time scales. For the evaluation, the Montana State University 3rd generation water vapor DIAL was modified to enable unattended operation for a period of several weeks. The performance of this V3.5 version DIAL was tested at MSU and NCAR in June and July of 2012. Further tests are currently in progress with Howard University at Beltsville, Maryland; and with the National Weather Service and Oklahoma University at Dallas/Fort Worth, Texas. The presentation will include a comparison of DIAL profiles against meteorological "truth" at the aforementioned locations including: radiosondes, Raman lidars, microwave and IR radiometers, AERONET and SUOMINET systems. Instrument reliability, uncertainty, systematic biases, detection height statistics, and environmental complications will be evaluated. Performance will be judged in the context of diverse scientific applications that range from operational weather prediction and seasonal climate variability, to more demanding climate system process studies at the land-canopy-ABL interface. Estimating the extent to which such research and operational applications can be satisfied with a low cost autonomous network of similar instruments is our principal objective.

  18. Quantum Statistical Behaviors of Interaction of an Atomic Bose-Einstein Condensate with Laser

    Institute of Scientific and Technical Information of China (English)

    YU Zhao-Xian; JIAO Zhi-Yong

    2001-01-01

    We have investigated quantum statistical behaviors of photons and atoms in interaction of an atomic Bose Einstein condensate with quantized laser field. When the quantized laser field is initially prepared in a superposition state which exhibits holes in its photon-number distribution, while the atomic field is initially in a Fock state, it is found that there is energy exchange between photons and atoms. For the input and output states, the photons and atoms may exhibit the sub-Poissonian distribution. The input and output laser fields may exhibit quadrature squeezing, but for the atomic field, only the output state exhibits quadrature squeezing. It is shown that there exists the violation of the Cauchy-Schwartz inequality, which means that the correlation between photons and atoms is nonclassical.``

  19. Atomically resolved surface structures of vapor deposited amorphous silicon-carbon alloys: An atomic force microscopy and spectroscopic study

    International Nuclear Information System (INIS)

    Silicon carbide alloys are widely used in high-tech applications due to their interesting combination of chemical, mechanical and electronic properties. Growing thin films of this material in a simple and controlled way is a hot topic in modern material's science. In particular, the possibility to tailor the film properties just by tuning the deposition temperature would be an important progress. In the present work amorphous silicon-carbon alloys thin films have been deposited by electron beam sublimation of a poly-crystalline silicon carbide target in vacuum environment. The deposition temperature was varied from Room Temperature to about 1300 K. The resulting films were analyzed by means of Ultra High Vacuum-Atomic Force Microscopy (UHV-AFM) down to even atomic resolution. The observed features agree with literature data, e.g. interatomic bond lengths, as achieved by others methods, and the structural arrangements of silicon and carbon atoms as concluded from IR and Raman spectroscopy measurements carried out on the same samples. The results not only allow a correlation between film properties and deposition temperature but also support the notion of the UHV-AFM images of the amorphous surfaces being atomically resolved.

  20. Optically pumped semiconductor lasers: Conception and characterization of a single mode source for Cesium atoms manipulation

    International Nuclear Information System (INIS)

    Lasers currently used in atomic clocks or inertial sensors are suffering from a lack of power, narrow linewidth or compactness for future spatial missions. Optically pumped semiconductor lasers, which combine the approach of classical solid state lasers and the engineering of semiconductor laser, are considered here as a candidate to a metrological laser source dedicated to the manipulation of Cesium atoms in these instruments. These lasers have demonstrated high power laser emission in a circular single transverse mode, as well as single longitudinal mode emission, favoured by the semiconductor structure and the external cavity design. We study the definition and the characterization of a proper semiconductor structure for the cooling and the detection of Cesium atoms at 852 nm. A compact and robust prototype tunable on the Cesium D2 hyperfine structure is built. The laser frequency is locked to an atomic transition thanks to a saturated absorption setup. The emission spectral properties are investigated, with a particular attention to the laser frequency noise and the laser linewidth. Finally, we describe and model the thermal properties of the semiconductor structure, which enables the simulation of the laser power characteristic. The experimental parameters are optimised to obtain the maximum output power with our structure. Thanks to our analysis, we propose several ways to overcome these limitations, by reducing the structure heating. (authors)

  1. Continuous-wave, single-frequency 229 nm laser source for laser cooling of cadmium atoms

    CERN Document Server

    Kaneda, Yushi; Merzlyak, Yevgeny; Yamaguchi, Atsushi; Hayashida, Keitaro; Ohmae, Noriaki; Katori, Hidetoshi

    2016-01-01

    Continuous-wave output at 229 nm for the application of laser cooling of Cd atoms was generated by the 4th harmonic using two successive second harmonic generation stages. Employing a single-frequency optically pumped semiconductor laser as a fundamental source, 0.56 W of output at 229 nm was observed with a 10-mm long, Brewster-cut BBO crystal in an external cavity with 1.62 W of 458 nm input. Conversion efficiency from 458 nm to 229 nm was more than 34%. By applying a tapered amplifier as a fundamental source, we demonstrated magneto-optical trapping of all stable Cd isotopes including isotopes $^{111}$Cd and $^{113}$Cd, which are applicable to optical lattice clocks.

  2. Frequency lock of a dye laser emission on iron atomic line top

    International Nuclear Information System (INIS)

    The aim of this thesis is to realize a frequency lock of a dye laser emission on iron atomic line top. To reach that goal, the author first presents the calculation of atomic vapour density by means of laser absorption ratio measure and studies the dye laser working. It is then necessary to find a device giving the required precision on the frequency of the absorption line choosen. It is obtained thanks to the atomic line reconstitution by optogalvanic effect which gives the reference. Besides, the author presents the necessity of a laser emission power regulation which is obtained thanks to a device including an acoustic and optic modulator. A reliable and accurate captor is choosen and adjusted testing various hollow cathode lamps. The method to obtain the frequency lock of laser emission on iron atomic line top is described. (TEC). 18 refs., 64 figs

  3. Pulsed carbon dioxide laser for cartilage vaporization and subchondral bone perforation in horses. Part II: Morphologic and histochemical reactions.

    Science.gov (United States)

    Nixon, A J; Krook, L P; Roth, J E; King, J M

    1991-01-01

    A pulsed carbon dioxide laser was used to vaporize articular cartilage in four horses, and perforate the cartilage and subchondral bone in four horses. Both intercarpal joints were examined arthroscopically and either a 1 cm cartilage crater or a series of holes was created in the third carpal bone of one joint. The contralateral carpus served as a control. After euthanasia at week 8, the treated and control joints were examined for gross changes, and samples of cartilage and subchondral bone, synovial membrane, and peripheral lymph nodes were examined histologically. Depletion of cartilage matrix glycosaminoglycan was assessed by safranin-O histochemical staining of the laser site and adjacent cartilage. Cartilage removal by laser vaporization resulted in rapid regrowth, with fibrous and fibrovascular tissue and occasional regions of fibrocartilage at week 8. The subchondral bone, synovial membrane, and draining lymph nodes appeared essentially unaffected by the laser cartilage vaporization procedure. Conversely, carbon dioxide laser drilling of subchondral bone resulted in poor penetration, extensive areas of thermal necrosis of bone, and significant secondary damage to the apposing articular surface of the radial carpal bone. PMID:1712998

  4. Determination of Mercury in Aqueous and Geologic Materials by Continuous Flow-Cold Vapor-Atomic Fluorescence Spectrometry (CVAFS)

    Science.gov (United States)

    Hageman, Philip L.

    2007-01-01

    New methods for the determination of total mercury in geologic materials and dissolved mercury in aqueous samples have been developed that will replace the methods currently (2006) in use. The new methods eliminate the use of sodium dichromate (Na2Cr2O7 ?2H2O) as an oxidizer and preservative and significantly lower the detection limit for geologic and aqueous samples. The new methods also update instrumentation from the traditional use of cold vapor-atomic absorption spectrometry to cold vapor-atomic fluorescence spectrometry. At the same time, the new digestion procedures for geologic materials use the same size test tubes, and the same aluminum heating block and hot plate as required by the current methods. New procedures for collecting and processing of aqueous samples use the same procedures that are currently (2006) in use except that the samples are now preserved with concentrated hydrochloric acid/bromine monochloride instead of sodium dichromate/nitric acid. Both the 'old' and new methods have the same analyst productivity rates. These similarities should permit easy migration to the new methods. Analysis of geologic and aqueous reference standards using the new methods show that these procedures provide mercury recoveries that are as good as or better than the previously used methods.

  5. Laser-induced fluorescence detection strategies for sodium atoms and compounds in high-pressure combustors

    Science.gov (United States)

    Weiland, Karen J. R.; Wise, Michael L.; Smith, Gregory P.

    1993-01-01

    A variety of laser-induced fluorescence schemes were examined experimentally in atmospheric pressure flames to determine their use for sodium atom and salt detection in high-pressure, optically thick environments. Collisional energy transfer plays a large role in fluorescence detection. Optimum sensitivity, at the parts in 10 exp 9 level for a single laser pulse, was obtained with the excitation of the 4p-3s transition at 330 nm and the detection of the 3d-3p fluorescence at 818 nm. Fluorescence loss processes, such as ionization and amplified spontaneous emission, were examined. A new laser-induced atomization/laser-induced fluorescence detection technique was demonstrated for NaOH and NaCl. A 248-nm excimer laser photodissociates the salt molecules present in the seeded flames prior to atom detection by laser-induced fluorescence.

  6. A compact and robust diode laser system for atom interferometry on a sounding rocket

    CERN Document Server

    Schkolnik, V; Wenzlawski, A; Grosse, J; Kohfeldt, A; Döringshoff, K; Wicht, A; Windpassinger, P; Sengstock, K; Braxmaier, C; Krutzik, M; Peters, A

    2016-01-01

    We present a diode laser system optimized for laser cooling and atom interferometry with ultra-cold rubidium atoms aboard sounding rockets as an important milestone towards space-borne quantum sensors. Design, assembly and qualification of the system, combing micro-integrated distributed feedback (DFB) diode laser modules and free space optical bench technology is presented in the context of the MAIUS (Matter-wave Interferometry in Microgravity) mission. This laser system, with a volume of 21 liters and total mass of 27 kg, passed all qualification tests for operation on sounding rockets and is currently used in the integrated MAIUS flight system producing Bose-Einstein condensates and performing atom interferometry based on Bragg diffraction. The MAIUS payload is being prepared for launch in fall 2016. We further report on a reference laser system, comprising a rubidium stabilized DFB laser, which was operated successfully on the TEXUS 51 mission in April 2015. The system demonstrated a high level of technol...

  7. Effects of carrier gas dynamics on single wall carbon nanotube chiral distributions during laser vaporization synthesis.

    Science.gov (United States)

    Landi, Brian J; Raffaelle, Ryne P

    2007-03-01

    We report on the utility of modifying the carrier gas dynamics during laser vaporization synthesis to alter the single wall carbon nanotube (SWNT) chiral distribution. SWNTs produced from an Alexandrite laser using conventional Ni/Co catalysts demonstrate marked differences in chiral distributions due to effects of helium gas and reactor chamber pressure, in comparison to conventional subambient pressures and argon gas. Optical absorption and Raman spectroscopies confirm that the SWNT diameter distribution decreases under higher pressure and with helium gas as opposed to argon. Fluorescence mapping of the raw soots in sodium dodecylbenzene sulfonate (SDBS)-D2O was used to estimate the relative (n, m)-SWNT content of the semiconducting types. A predominance of type II structures for each synthesis condition was observed. The distribution of SWNT chiral angles was observed to shift away from near-armchair configurations under higher pressure and with helium gas. These results illustrate the importance of gas type and pressure on the condensation/cooling rate, which allows for synthesis of specific SWNT chiral distributions. PMID:17450850

  8. Differential mobility analysis of nanoparticles generated by laser vaporization and controlled condensation (LVCC)

    International Nuclear Information System (INIS)

    Silicon and iron aluminide (FeAl) nanoparticles were synthesized by a laser vaporization controlled condensation (LVCC) method. The particles generated by the laser ablation of solid targets were transported and deposited in the presence of well-defined thermal and electric field in a newly designed flow-type LVCC chamber. The deposition process of nanoparticles was controlled by the balance of the external forces; i.e., gas flow, thermophoretic and electrostatic forces. The size distributions of generated nanoparticles were analyzed using a low-pressure differential mobility analyzer (LP-DMA). The effect of synthesis condition on the size distribution was analyzed by changing the pressure of the carrier gas (20-200 Torr), the temperature gradient in the LVCC chamber (ΔT=0-190 deg. C) and the electric field applied between the LVCC chamber plates (E=0-3000 V/m). It was found that electrostatic field was effective to selectively deposit small size nanoparticles (about 10 nm) with expelling large droplet-like particles

  9. THE SPECTROSCOPY OF URANIUM ATOM WITHIN THE "SILVA" PROGRAM

    OpenAIRE

    Avril, R.; Ebrardt, J.; Petit, A.; Viala, F.; Vors, E.

    1987-01-01

    Atomic vapor laser isotope separation (SILVA) has been recognized as beeing an attractive powerful technique for the enrichment of uranium for light water reactor fuel. Since the heart of the AVLIS process is based on selective multistep photoionization of an uranium atomic vapor stream, the development of this process in France, has stimulated intensive studies in the field of uranium spectroscopy.

  10. Studies of atomic processes for x-ray lasers and x-ray sources

    International Nuclear Information System (INIS)

    A computer tool for displaying Grotrian diagram of atomic energy level structure is developed, which uses computed atomic data from the HULLAC code. This tool is intended for providing atomic data of complex multiply charged ions for modeling x-ray lasers and x-ray sources. Visualization of the atomic structure using the Grotrian tool appears to be useful for identifying dominant ionization/excitation processes and emission channels in the plasma. (author)

  11. Time-resolved ionization of the hydrogen atom in strong laser fields

    International Nuclear Information System (INIS)

    We use the strong field approximation to study the single-photon ionization of the hydrogen atom in the time domain. During the interaction of the laser pulse and the atom, the electron is pumped to the Volkov state and has a widely energy distribution at the beginning of the laser pulse. With the time evolution, only the photon-electron with the energy hra - Ip is survived, where to is the laser angular frequency, and Ip is the ionization potential of the atom. Therefore we observed how the energy spectrum of the ionized electron builds in the time domain.

  12. Chemical oxygen-iodine laser with atomic iodine generated in a separate reactor

    Czech Academy of Sciences Publication Activity Database

    Špalek, Otomar; Jirásek, Vít; Čenský, Miroslav; Kodymová, Jarmila; Picková, Irena; Jakubec, Ivo

    Bellingham: SPIE, 2006 - (Phipps, C.), 62611T/1-62611T/10. (Proceedings of SPIE. 6261). ISBN 0-8194-6326-4. ISSN 0277-786X. [High-Power Laser Ablation /6./. Taos, New Mexico (US), 07.05.2006-12.05.2006] R&D Projects: GA ČR GA202/05/0359 Grant ostatní: USAF EOARD(US) FA8655-02-M4040 Institutional research plan: CEZ:AV0Z10100523; CEZ:AV0Z40320502 Keywords : atomic iodine * atomic chlorine * atomic fluorine * chemical oxygen-iodine laser * COIL Subject RIV: BH - Optics, Masers, Lasers

  13. A self-injected, diode-pumped, solid-state ring laser for laser cooling of Li atoms

    International Nuclear Information System (INIS)

    We have constructed a solid-state light source for experiments with laser cooled lithium atoms based on a Nd:Y V O4 ring laser with second-harmonic generation. Unidirectional lasing, an improved mode selection, and a high output power of the ring laser were achieved by weak coupling to an external cavity which contained the lossy elements required for single frequency operation. Continuous frequency tuning is accomplished by controlling two piezoelectric transducers (PZTs) in the internal and the external cavities simultaneously. The light source has been utilized to trap and cool fermionic lithium atoms into the quantum degenerate regime

  14. A self-injected, diode-pumped, solid-state ring laser for laser cooling of Li atoms

    Energy Technology Data Exchange (ETDEWEB)

    Miake, Yudai; Mukaiyama, Takashi, E-mail: muka@ils.uec.ac.jp [Institute for Laser Science, University of Electro-Communications, 1-5-1 Chofugaoka, Chofu, Tokyo 182-8585 (Japan); O’Hara, Kenneth M. [Department of Physics, The Pennsylvania State University, University Park, Pennsylvania 16802-6300 (United States); Gensemer, Stephen [CSIRO Manufacturing Flagship, Lindfield, NSW 2070 (Australia)

    2015-04-15

    We have constructed a solid-state light source for experiments with laser cooled lithium atoms based on a Nd:Y V O{sub 4} ring laser with second-harmonic generation. Unidirectional lasing, an improved mode selection, and a high output power of the ring laser were achieved by weak coupling to an external cavity which contained the lossy elements required for single frequency operation. Continuous frequency tuning is accomplished by controlling two piezoelectric transducers (PZTs) in the internal and the external cavities simultaneously. The light source has been utilized to trap and cool fermionic lithium atoms into the quantum degenerate regime.

  15. A self-injected, diode-pumped, solid-state ring laser for laser cooling of Li atoms

    Science.gov (United States)

    Miake, Yudai; Mukaiyama, Takashi; O'Hara, Kenneth M.; Gensemer, Stephen

    2015-04-01

    We have constructed a solid-state light source for experiments with laser cooled lithium atoms based on a Nd:Y V O4 ring laser with second-harmonic generation. Unidirectional lasing, an improved mode selection, and a high output power of the ring laser were achieved by weak coupling to an external cavity which contained the lossy elements required for single frequency operation. Continuous frequency tuning is accomplished by controlling two piezoelectric transducers (PZTs) in the internal and the external cavities simultaneously. The light source has been utilized to trap and cool fermionic lithium atoms into the quantum degenerate regime.

  16. Visible laser discharge studies. Quarterly progress report, June 1, 1977--August 31, 1977. [CdHg vapors

    Energy Technology Data Exchange (ETDEWEB)

    Srivastava, B N; Jacob, J H; Mangano, J A

    1977-01-01

    In order to facilitate the development of metal vapor excimer lasers for inertial fusion, a theoretical study has been undertaken to identify the dominant discharge physics and kinetics for metal vapor excimers like cadmium-mercury (CdHg). Interest in such lasers have been heightened since the reported observation of gain in CdHg. An efficient method of pumping the first excited state of metal vapors is by secondary electrons created in a discharge. By discharge pumping it is possible to create mainly the lowest excited state, thereby minimizing highly excited electronic states that could photoabsorb. E-beam pumping may have difficulty in pumping metal vapor excimers due to photoabsorption by excited species. To obtain high efficiencies for CdHg system by discharge pumping three technical issues must be addressed: (1) inefficiencies in discharge pumping due to energy flow into excited states; (2) discharge stability; and (3) efficient discharge enhancement. The present effort is directed to the above issues through the development of a kinetics code that models the dominant kinetics of CdHg laser system. The bulk of the report is devoted to identification of inefficiencies in discharge pumping due to energy flow into excited states. The analysis can also be used to predict discharge stability and discharge enhancement.

  17. Multiphoton resonant ionization of hydrogen atom exposed to two-colour laser pulses

    International Nuclear Information System (INIS)

    This paper studies the multiphoton resonant ionization by two-colour laser pulses in the hydrogen atom by solving the time-dependent Schrodinger equation. By fixing the parameters of fundamental laser field and scanning the frequency of second laser field, it finds that the ionization probability shows several resonance peaks and is also much larger than the linear superposition of probabilities by applying two lasers separately. The enhancement of the ionization happens when the system is resonantly pumped to the excited states by absorbing two or more colour photons non-sequentially. (atomic and molecular physics)

  18. Coherent population transfer in Rydberg potassium atom by a single frequency-chirped laser pulse

    Institute of Scientific and Technical Information of China (English)

    Zhang Xian-Zhou; Ma Qiao-Zhi; Li Xiao-Hong

    2006-01-01

    By using the time-dependent multilevel approach, we have calculated the coherent population transfer among the quantum states of potassium atom by a single frequency-chirped laser pulse. The results show that the population can be efficiently transferred to a target state and be trapped there by using an ‘intuitive’ or a ‘counter-intuitive’ frequency sweep laser pulse in the case of ‘narrowband’ frequency-chirped laser pulse. It is also found that a pair of sequential ‘broadband’ frequency-chirped laser pulses can efficiently transfer population from one ground state of the A atom to the other one.

  19. Laser agitates probability flow in atoms to form alternating current and its peak-dip phenomenon

    CERN Document Server

    Cui, Huai-Yang

    2016-01-01

    By using trajectory-based approaches to quantum transition, it is found that laser can agitate the probability flow in atoms to form alternating current with the frequency of the laser. The detailed physical process of quantum transition is investigated, during which the alternating current in atomic probability flow becomes a key role connecting the external electromagnetic wave with the evolution of the quantum states in atoms. Computer was employed to simulate the physical process. The atomic alternating current may have the peak-dip phenomenon.

  20. Charge states of high Z atoms in a strong laser field

    International Nuclear Information System (INIS)

    We present a numerical solution of the Thomas-Fermi atom in the presence of a static electric field as a model of the adiabatic response of a heavy atom in the presence of a strong laser field. In this semiclassical approach, we calculate the resulting charge state of the atom and its induced dipole moment after the field is turned on. Due to the scaling properties of the Thomas-Fermi approach, the resulting total atomic charge and dipole moment can be expressed as a universal function of the field. We compare our results with recent ionization experiments performed on noble gases using laser fields. 7 refs., 5 figs

  1. Proposed search for an electric-dipole moment using laser-cooled $^{171}$Yb atoms

    OpenAIRE

    Natarajan, Vasant

    2005-01-01

    We propose an experiment to search for a permanent atomic electric-dipole moment (EDM) using laser-cooled $^{171}$Yb atoms launched in an atomic fountain. A uniform B field sets the quantization axis, and the Ramsey separated-oscillatory-fields method is used to measure the Zeeman precession frequency of the atoms. Laser beams of appropriate polarization are used for preparation and detection in a given magnetic sublevel. The signature of an EDM is a shift in the Ramsey resonance correlated w...

  2. Design and Fabrication of a Chip-based Continuous-wave Atom Laser

    OpenAIRE

    Power, E. P.; George, L; Vanderelzen, B.; Herrera-Fierro, P.; Murphy, R; Yalisove, S. M.; Raithel, G.

    2012-01-01

    We present a design for a continuous-wave (CW) atom laser on a chip and describe the process used to fabricate the device. Our design aims to integrate quadrupole magnetic guiding of ground state Rb atoms with continuous surface adsorption evaporative cooling to create a continuous Bose-Einstein condensate; out-coupled atoms from the condensate should realize a CW atom laser. We choose a geometry with three wires embedded in a spiral pattern in a silicon subtrate. The guide features an integr...

  3. Tissue ablation after 120W greenlight laser vaporization and bipolar plasma vaporization of the prostate: a comparison using transrectal three-dimensional ultrasound volumetry

    Science.gov (United States)

    Kranzbühler, Benedikt; Gross, Oliver; Fankhauser, Christian D.; Hefermehl, Lukas J.; Poyet, Cédric; Largo, Remo; Müntener, Michael; Seifert, Hans-Helge; Zimmermann, Matthias; Sulser, Tullio; Müller, Alexander; Hermanns, Thomas

    2012-02-01

    Introduction and objectives: Greenlight laser vaporization (LV) of the prostate is characterized by simultaneous vaporization and coagulation of prostatic tissue resulting in tissue ablation together with excellent hemostasis during the procedure. It has been reported that bipolar plasma vaporization (BPV) of the prostate might be an alternative for LV. So far, it has not been shown that BPV is as effective as LV in terms of tissue ablation or hemostasis. We performed transrectal three-dimensional ultrasound investigations to compare the efficiency of tissue ablation between LV and BPV. Methods: Between 11.2009 and 5.2011, 50 patients underwent pure BPV in our institution. These patients were matched with regard to the pre-operative prostate volume to 50 LV patients from our existing 3D-volumetry-database. Transrectal 3D ultrasound and planimetric volumetry of the prostate were performed pre-operatively, after catheter removal, 6 weeks and 6 months. Results: Median pre-operative prostate volume was not significantly different between the two groups (45.3ml vs. 45.4ml; p=1.0). After catheter removal, median absolute volume reduction (BPV 12.4ml, LV 6.55ml) as well as relative volume reduction (27.8% vs. 16.4%) were significantly higher in the BPV group (pablation with initial prostatic swelling. BPV seems to be superior due to a higher relative volume reduction. This difference had no clinical impact after a follow-up of 6M.

  4. Novel laser atomic fluorescence spectrometer for environmental and biomedical analyses of heavy metals

    Science.gov (United States)

    Dergachev, Alex Y.; Mirov, Sergey B.; Pitt, Robert E.; Parmer, Keith D.

    1997-05-01

    We report on the development of a novel experimental set-up using laser atomic fluorescence for detection and concentration measurements of heavy metal atoms for environmental and biomedical analyses. This spectrometer is based on the application of tunable LiF:F2+** and LiF:F2- color center and alexandrite lasers with nonlinear converters for narrowband excitation of atomic fluorescence and the use of gated multichannel CCD detectors for fluorescence measurements. A standard graphite furnace module was used for sample atomization. The laser sources used provide narrowband selective laser excitation continuously tunable in the 200 - 400 nm range and are therefore suitable for resonant excitation of atomic transitions in practically all known heavy metal atoms. In the first experiments, water samples containing Cu, Pb and Fe impurities were studied and detection levels of less than 1 ppb were observed. Comparison of the results of atomic laser fluorescence analysis and traditional atomic absorption spectrometry showed good qualitative agreement between these two methods. It is projected that full optimization of our experimental set up will allow for improved detection levels of several orders of magnitude. Possible optimization and simplification of the spectrometer are discussed in the context of developing a portable instrument for field use.

  5. Inversion symmetry breaking of atomic bound states in strong and short laser fields

    CERN Document Server

    Stooß, Veit; Ott, Christian; Blättermann, Alexander; Ding, Thomas; Pfeifer, Thomas

    2015-01-01

    In any atomic species, the spherically symmetric potential originating from the charged nucleus results in fundamental symmetry properties governing the structure of atomic states and transition rules between them. If atoms are exposed to external electric fields, these properties are modified giving rise to energy shifts such as the AC Stark-effect in varying fields and, contrary to this in a constant (DC) electric field for high enough field strengths, the breaking of the atomic symmetry which causes fundamental changes in the atom's properties. This has already been observed for atomic Rydberg states with high principal quantum numbers. Here, we report on the observation of symmetry breaking effects in Helium atoms for states with principal quantum number n=2 utilizing strong visible laser fields. These findings were enabled by temporally resolving the dynamics better than the sub-optical cycle of the applied laser field, utilizing the method of attosecond transient absorption spectroscopy (ATAS). We ident...

  6. Chemical vapor generation of silver for atomic absorption spectrometry with the multiatomizer: Radiotracer efficiency study and characterization of silver species

    International Nuclear Information System (INIS)

    Volatile Ag species were generated in flow injection arrangement from nitric acid environment in the presence of surfactants (Triton X-100 and Antifoam B) and permanent Pd deposits as the reaction modifiers. Atomic absorption spectrometry (AAS) with multiple microflame quartz tube atomizer heated to 900 deg. C was used for atomization; evidence was found for thermal mechanism of atomization. Relative and absolute limits of detection (3σ, 250 μl sample loop) measured under optimized conditions were: 1.4 μg l-1 and 0.35 ng, respectively. The efficiency of chemical vapor generation (CVG) as well as spatial distribution of residual analyte in the apparatus was studied by 111Ag radioactive indicator (half-life 7.45 days) of high specific activity. It was found out that 23% of analyte was released into the gaseous phase. However, only 8% was found on filters placed at the entrance to the atomizer due to transport losses. About 40% of analyte remained in waste liquid, whereas the rest was found deposited over the CVG system. Presented study follows the hypothesis that the 'volatile' Ag species are actually metallic nanoparticles formed upon reduction in liquid phase and then released with good efficiency to the gaseous phase. Number/charge size distributions of dry aerosol were determined by Scanning Mobility Particle Sizer. Ag was detected in 40-45 nm particles holding 10 times more charge if compared to Boltzmann equilibrium. At the same time, Ag was also present on 150 nm particles, the main size mode of the CVG generator. The increase of Ag in standards was reflected by proportional increase in particle number/charge for 40-45 nm size particles only. Transmission electron microscopy revealed particles of 8 ± 2 nm sampled from the gaseous phase, which were associated in isolated clusters of few to few tens of nanometres. Ag presence in those particles was confirmed by Energy Dispersive X-ray Spectroscopy (EDS) analysis.

  7. Collisions of metastable Ne*, He* atoms with ground-state He, Ne atoms studied by atomic beam and laser techniques

    International Nuclear Information System (INIS)

    A crossed nozzle-beam experiment is used to investigate thermal energy collisions: Ne* (2p53s, 3P0,2) + He(1s2, 1S0), almost purely elastic, and He*(1s2s, 1,3S + Ne(2p6, 1S0), in which inelastic excitation transfers occur. State and velocity selection of the scattered Ne* atoms is performed using a tunable cw dye laser frequency locked on a definite Zeeman component of the transition 1s5 → 2p6 (λ = 614.3 nm) of 20Ne or 22Ne. In the purely elastic case, this technique allows the selection of one of the two final velocities, and then an unambiguous transformation of the differential cross section at 62 meV tallies on accords with a calculation using a single effective potential. In He* on Ne collisions, the main inelastic processes are endothermic excitation transfers from He*(21S). Experimental results obtained at different energies (62, 95, 109, 124 meV) show that the transfers essentially result in levels 3s and 4d of Ne. (orig.)

  8. High-order harmonic generation from Rydberg atoms driven by plasmonic-enhanced laser fields

    CERN Document Server

    Tikman, Y; Ciappina, M F; Chacon, A; Altun, Z; Lewenstein, M

    2015-01-01

    We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed certain threshold in order to generate HHG, when noble gas atoms in their ground state are used as an active medium. One way to enhance the coherent light coming from a conventional laser oscillator is to take advantage of the amplification obtained by the so-called surface plasmon polaritons, created when a low intensity laser field is focused onto a metallic nanostructure. The main limitation of this scheme is the low damage threshold of the materials employed in the nanostructures engineering. In this work we propose to use Rydberg atoms, driven by spatially inhomogeneous, plasmonic-enhanced laser fields, for HHG. We exhaustively discuss the behaviour and efficiency of these systems in the generation of coherent harmonic emission. To this aim we numerically solve the time...

  9. Role of atomic hydrogen density and energy in low power chemical vapor deposition synthesis of diamond films

    International Nuclear Information System (INIS)

    Polycrystalline diamond films were synthesized on silicon substrates without diamond seeding by a very low power (∼40-80 W) microwave plasma continuous vapor deposition reaction of a mixture of helium-hydrogen-methane (48.2/48.2/3.6%) or argon-hydrogen-methane (17.5/80/2.5%). However, predominantly graphitic carbon films or no films formed when neon, krypton, or xenon was substituted for helium or argon. The films were characterized by time of flight secondary ion mass spectroscopy, X-ray photoelectron spectroscopy, Raman spectroscopy, scanning electron microscopy, and X-ray diffraction. It is proposed that each of He+ and Ar+ served as a catalyst with atomic hydrogen to form an energetic plasma since only plasmas having these ions in the presence of atomic hydrogen showed significantly broadened H α lines corresponding to an average hydrogen atom temperature of >100 eV as reported previously. It was found that not only the energy, but also the H density uniquely increases in He-H2 and Ar-H2 plasmas. Bombardment of the carbon surface by highly energetic hydrogen formed by the catalysis reaction may play a role in the formation of diamond. Then, by this novel pathway, the relevance of the CO tie line is eliminated along with other stringent conditions and complicated and inefficient techniques which limit broad application of the versatility and superiority of diamond thin film technology

  10. A highly sensitive method for the determination of mercury using vapor generation gold wire microextraction and electrothermal atomic absorption spectrometry

    International Nuclear Information System (INIS)

    The study introduces a new simple and highly sensitive method for headspace solid phase microextraction (HS-SPME) coupled with electrothermal atomic absorption spectrometric determination of mercury. In the proposed method, a gold wire, mounted in the headspace of a sample solution in a sealed bottle, is used for collection of mercury vapor generated by addition of sodium tetrahydroborate. The gold wire is then simply inserted in the sample introduction hole of a graphite furnace of an electrothermal atomic absorption spectrometry instrument. By applying an atomization temperature of 600 deg. C, mercury is rapidly desorbed from the wire and determined with high sensitivity. Factorial design and response surface analysis methods were used for optimization of the effect of five different variables in order to maximize the mercury signal. By using a 0.75 mm diameter gold wire, a sample volume of about 8 ml and an extraction time of 11 min, the sensitivity of mercury determination was enhanced up to 104 times in comparison to its ordinary ETAAS determination with direct injection of 10 μl sample solutions. A detection limit of 0.006 ng ml-1 and a precision better than 4.6% (relative standard deviation) were obtained. The method was successfully applied to the determination of mercury in industrial wastewaters and tuna fish samples

  11. A highly sensitive method for the determination of mercury using vapor generation gold wire microextraction and electrothermal atomic absorption spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    Hashemi, Payman [Department of Chemistry, Lorestan University, Khorram Abad (Iran, Islamic Republic of)], E-mail: payman_hashemi@yahoo.com; Rahimi, Akram [Department of Chemistry, Lorestan University, Khorram Abad (Iran, Islamic Republic of)

    2007-04-15

    The study introduces a new simple and highly sensitive method for headspace solid phase microextraction (HS-SPME) coupled with electrothermal atomic absorption spectrometric determination of mercury. In the proposed method, a gold wire, mounted in the headspace of a sample solution in a sealed bottle, is used for collection of mercury vapor generated by addition of sodium tetrahydroborate. The gold wire is then simply inserted in the sample introduction hole of a graphite furnace of an electrothermal atomic absorption spectrometry instrument. By applying an atomization temperature of 600 deg. C, mercury is rapidly desorbed from the wire and determined with high sensitivity. Factorial design and response surface analysis methods were used for optimization of the effect of five different variables in order to maximize the mercury signal. By using a 0.75 mm diameter gold wire, a sample volume of about 8 ml and an extraction time of 11 min, the sensitivity of mercury determination was enhanced up to 10{sup 4} times in comparison to its ordinary ETAAS determination with direct injection of 10 {mu}l sample solutions. A detection limit of 0.006 ng ml{sup -1} and a precision better than 4.6% (relative standard deviation) were obtained. The method was successfully applied to the determination of mercury in industrial wastewaters and tuna fish samples.

  12. A low phase noise microwave frequency synthesis for a high-performance cesium vapor cell atomic clock

    International Nuclear Information System (INIS)

    We report the development, absolute phase noise, and residual phase noise characterization of a 9.192 GHz microwave frequency synthesis chain devoted to be used as a local oscillator in a high-performance cesium vapor cell atomic clock based on coherent population trapping (CPT). It is based on frequency multiplication of an ultra-low phase noise 100 MHz oven-controlled quartz crystal oscillator using a nonlinear transmission line-based chain. Absolute phase noise performances of the 9.192 GHz output signal are measured to be −42, −100, −117 dB rad2/Hz and −129 dB rad2/Hz at 1 Hz, 100 Hz, 1 kHz, and 10 kHz offset frequencies, respectively. Compared to current results obtained in a state-of-the-art CPT-based frequency standard developed at LNE-SYRTE, this represents an improvement of 8 dB and 10 dB at f = 166 Hz and f = 10 kHz, respectively. With such performances, the expected Dick effect contribution to the atomic clock short term frequency stability is reported at a level of 6.2 × 10−14 at 1 s integration time, that is a factor 3 higher than the atomic clock shot noise limit. Main limitations are pointed out

  13. Direct determination of mercury in white vinegar by matrix assisted photochemical vapor generation atomic fluorescence spectrometry detection

    Energy Technology Data Exchange (ETDEWEB)

    Liu Qingyang, E-mail: liuqingyang0807@yahoo.com.c [Beijing Center for Physical and Chemical Analysis, Beijing 100089 (China)

    2010-07-15

    This paper proposes the use of photochemical vapor generation with acetic acid as sample introduction for the direct determination of ultra-trace mercury in white vinegars by atomic fluorescence spectrometry. Under ultraviolet irradiation, the sample matrix (acetic acid) can reduce mercury ion to atomic mercury Hg{sup 0}, which is swept by argon gas into an atomic fluorescence spectrometer for subsequent analytical measurements. The effects of several factors such as the concentration of acetic acid, irradiation time, the flow rate of the carrier gas and matrix effects were discussed and optimized to give detection limits of 0.08 ng mL{sup -1} for mercury. Using the experimental conditions established during the optimization (3% v/v acetic acid, 30 s irradiation time and 20 W mercury lamp), the precision levels, expressed as relative standard deviation, were 4.6% (one day) and 7.8% (inter-day) for mercury (n = 9). Addition/recovery tests for evaluation of the accuracy were in the range of 92-98% for mercury. The method was also validated by analysis of vinegar samples without detectable amount of Hg spiked with aqueous standard reference materials (GBW(E) 080392 and GBW(E) 080393). The results were also compared with those obtained by acid digestion procedure and determination of mercury by ICP-MS. There was no significant difference between the results obtained by the two methods based on a t-test (at 95% confidence level).

  14. Process development for the manufacture of an integrated dispenser cathode assembly using laser chemical vapor deposition

    Science.gov (United States)

    Johnson, Ryan William

    2005-07-01

    Laser Chemical Vapor Deposition (LCVD) has been shown to have great potential for the manufacture of small, complex, two or three dimensional metal and ceramic parts. One of the most promising applications of the technology is in the fabrication of an integrated dispenser cathode assembly. This application requires the deposition of a boron nitride-molybdenum composite structure. In order to realize this structure, work was done to improve the control and understanding of the LCVD process and to determine experimental conditions conducive to the growth of the required materials. A series of carbon fiber and line deposition studies were used to characterize process-shape relationships and study the kinetics of carbon LCVD. These studies provided a foundation for the fabrication of the first high aspect ratio multi-layered LCVD wall structures. The kinetics studies enabled the formulation of an advanced computational model in the FLUENT CFD package for studying energy transport, mass and momentum transport, and species transport within a forced flow LCVD environment. The model was applied to two different material systems and used to quantify deposition rates and identify rate-limiting regimes. A computational thermal-structural model was also developed using the ANSYS software package to study the thermal stress state within an LCVD deposit during growth. Georgia Tech's LCVD system was modified and used to characterize both boron nitride and molybdenum deposition independently. The focus was on understanding the relations among process parameters and deposit shape. Boron nitride was deposited using a B3 N3H6-N2 mixture and growth was characterized by sporadic nucleation followed by rapid bulk growth. Molybdenum was deposited from the MoCl5-H2 system and showed slow, but stable growth. Each material was used to grow both fibers and lines. The fabrication of a boron nitride-molybdenum composite was also demonstrated. In sum, this work served to both advance the

  15. Laser cooling of single trapped atoms to the ground state: a dark state in position space

    OpenAIRE

    Morigi, Giovanna; Cirac Sasturáin, Juan Ignacio,; Ellinger, K; Zoller, P.

    1997-01-01

    We propose a scheme that allows us to laser cool trapped atoms to the ground state of a one-dimensional confining potential. The scheme is based on the creation of a dark state by designing the laser profile, so that the hottest atoms are coherently pumped to another internal level, and then repumped back. The scheme works beyond the Lamb-Dicke limit. We present results of a full quantum treatment for a one-dimensional model.

  16. Studies of atomic processes for x-ray lasers and x-ray sources

    International Nuclear Information System (INIS)

    An integrated system of computational atomic database for spectroscopic investigation of x-ray lasers and x-ray sources is developed. The system consists of atomic data codes, database, a collisional radiative code, and programs for visualizing spectrum. Gain of Ni-like La laser is analyzed using the model. Furthermore, EUV spectrum from Xe is investigated, to identify measured transition arrays in 10 nm to 16 nm for the EUV light source. (author)

  17. Pulsed carbon dioxide laser for cartilage vaporization and subchondral bone perforation in horses. Part I: Technique and clinical results.

    Science.gov (United States)

    Roth, J E; Nixon, A J; Gantz, V A; Meyer, D; Mohammed, H

    1991-01-01

    A carbon dioxide laser, used in a rapidly pulsed mode, was evaluated for intra-articular use in horses. Under arthroscopic guidance, a lensed 5 mm laser probe attached directly to a hand-held carbon dioxide laser was inserted into one intercarpal joint of eight horses. In four horses, a cartilage crater 1 cm in diameter was created to the level of the subchondral bone of the articular surface of the third carpal bone. In four horses, the laser was directed perpendicular to the articular surface of the third carpal bone and activated to penetrate the cartilage and subchondral bone. The intercarpal joint of the opposite carpus in each horse was subjected to arthroscopic examination and insertion of the laser probe for an equivalent time. The laser was not activated and these joints served as sham operated controls. The horses were evaluated clinically for 8 weeks, then euthanatized, and the joints were examined radiographically, grossly, and histologically. Pulsed carbon dioxide laser vaporized cartilage readily but penetrated bone poorly. Cartilage vaporization resulted in no greater swelling, heat, pain on flexion, lameness, or synovial fluid reaction than the sham procedure. Laser drilling resulted in a shallow, charred hole with a tenacious carbon residue, and in combination with the thermal damage to deeper bone, resulted in increased swelling, mild lameness and a low-grade, but persistent synovitis. The carbon dioxide laser is a useful intra-articular instrument for removal of cartilage and has potential application in inaccessible regions of diarthrodial joints. It does not penetrate bone sufficiently to have application in subchondral drilling. PMID:1853552

  18. Coherent Population Trapping Resonances in Cs Atomic Vapor Layers of Micrometric Thickness

    Directory of Open Access Journals (Sweden)

    A. Krasteva

    2011-01-01

    Full Text Available We report on a novel behavior of the electromagnetically induced absorption (EIA resonance observed on the D2 line of Cs for atoms confined in cells with micrometric thickness. With the enhancement of light intensity, the EIA resonance amplitude suffers from fast reduction, and even at very low intensity (W < 1 mW/cm2, resonance sign reversal takes place and electromagnetically induced transparency (EIT resonance is observed. Similar EIA resonance transformation to EIT one is not observed in conventional cm-size cells. A theoretical model is proposed to analyze the physical processes behind the EIA resonance sign reversal with light intensity. The model involves elastic interactions between Cs atoms as well as elastic interaction of atom micrometric-cell windows, both resulting in depolarization of excited state which can lead to the new observations. The effect of excited state depolarization is confirmed also by the fluorescence (absorption spectra measurement in micrometric cells with different thicknesses.

  19. Making custom fiber lasers for use in an atomic physics experiment

    Science.gov (United States)

    Khademian, Ali; Cameron, Garnet; Nault, Kyla; Shiner, David

    2016-05-01

    Fiber lasers can be a reasonable choice for a laser source in atomic physics. Our particular applications involve the optical pumping and in some applications cooling of various transitions in atomic helium. Doped fiber with emission at the required wavelengths is necessary. Readily available fiber and approximate wavelength emission ranges include Yb (990 - 1150 nm), Er/Yb (1530 - 1625 nm) and Th (1900 -2100 nm). High efficiency conversion of pump photons into stable single frequency laser emission at the required wavelength is the function of the fiber laser. A simple fiber laser cavity uses a short (~ few mm) fiber grating high reflector mirror, a doped fiber section for the laser cavity, and a long (~ few cm) fiber grating output coupler. To ensure reliable single frequency operation, the laser cavity length should be within 2-3 times the output grating length. However the cavity length must be long enough for round trip gains to compensate for the output mirror transmission loss. Efficiency can be maximized by avoiding fiber splices in the fiber laser cavity. This requires that the gratings be written into the doped fiber directly. In our previous designs, back coupling of the fiber laser into the pump laser contributes to instability and sometimes caused catastrophic pump failure. Current designs use a fiber based wavelength splitter (WDM) to study and circumvent this problem. Data will be presented on the fiber lasers at 1083 nm. Work on a Thulium 2057 nm fiber laser will also be discussed. This work is supported by NSF Grant # 1404498.

  20. Analysis of Amphiphilic Lipids and Hydrophobic Proteins Using Nonresonant Femtosecond Laser Vaporization with Electrospray Post-Ionization

    Science.gov (United States)

    Brady, John J.; Judge, Elizabeth J.; Levis, Robert J.

    2011-04-01

    Amphiphilic lipids and hydrophobic proteins are vaporized at atmospheric pressure using nonresonant 70 femtosecond (fs) laser pulses followed by electrospray post-ionization prior to being transferred into a time-of-flight mass spectrometer for mass analysis. Measurements of molecules on metal and transparent dielectric surfaces indicate that vaporization occurs through a nonthermal mechanism. The molecules analyzed include the lipids 1-monooleoyl-rac-glycerol, 1,2-dihexanoyl- sn-glycero-3-phosphocholine, 1,2-dimyristoyl- sn-glycero-3-phosphocholine, and the hydrophobic proteins gramicidin A, B, and C. Vaporization of lipids from blood and milk are also presented to demonstrate that lipids in complex systems can be transferred intact into the gas phase for mass analysis.

  1. Determination of trace mercury in environmental samples by cold vapor atomic fluorescence spectrometry after cloud point extraction

    International Nuclear Information System (INIS)

    A sensitive method is presented for the determination of ultra-trace levels of mercury using cold vapor atomic fluorescence spectrometry along with cloud point extraction. Preconcentration is based on the complexation of Hg(II) by dithizone, followed by micelle-mediated extraction of the complex using the surfactant Triton X-114. Foaming, which is always observed when generating vapor mercury in the presence of surfactant, was strongly reduced by using SnCl2 as a reducing reagent, and a homemade gas-liquid separator. Variables that affect the assay were optimized. These included pH value, concentration of chelating reagent, concentration of Triton X-114, equilibration temperature and time. The preconcentration of a 45-mL sample gave an enhancement factor of 29. The calibration graph is linear in the range from 0. 05 to 5. 0 ng mL-1 with a correlation coefficient of 0. 9991. The limit of detection obtained under the optimal conditions is 5 pg mL-1. The relative standard deviation for seven replicate determinations at 0. 5 ng mL-1 level is 5. 2%. The method was successfully applied to the determination of Hg in real samples. (author)

  2. Mercury determination in non- and biodegradable materials by cold vapor capacitively coupled plasma microtorch atomic emission spectrometry

    International Nuclear Information System (INIS)

    Highlights: → Use of a miniaturized analytical system with microtorch plasma for Hg determination. → Determination of Hg in non- and biodegradable materials using cold vapor generation. → Figures of merit and advantages of the miniaturized system for Hg determination. - Abstract: A new analytical system consisting of a low power capacitively coupled plasma microtorch (20 W, 13.56 MHz, 150 ml min-1 Ar) and a microspectrometer was investigated for the Hg determination in non- and biodegradable materials by cold-vapor generation, using SnCl2 reductant, and atomic emission spectrometry. The investigated miniaturized system was used for Hg determination in recyclable plastics from electronic equipments and biodegradable materials (shopping bags of 98% biodegradable polyethylene and corn starch) with the advantages of easy operation and low analysis costs. Samples were mineralized in HNO3-H2SO4 mixture in a high-pressure microwave system. The detection limits of 0.05 ng ml-1 or 0.08 μg g-1 in solid sample were compared with those reported for other analytical systems. The method precision was 1.5-9.4% for Hg levels of 1.37-13.9 mg kg-1, while recovery in two polyethylene certified reference materials in the range 98.7 ± 4.5% (95% confidence level).

  3. Quasistatic limit of the strong-field approximation describing atoms in intense laser fields: Circular polarization

    CERN Document Server

    Bauer, J H

    2010-01-01

    In the recent work of Vanne and Saenz [Phys. Rev. A 75, 063403 (2007)] the quasistatic limit of the velocity gauge strong-field approximation describing the ionization rate of atomic or molecular systems exposed to linearly polarized laser fields was derived. It was shown that in the low-frequency limit the ionization rate is proportional to the laser frequency (for a constant intensity of the laser field). In the present work I show that for circularly polarized laser fields the ionization rate is proportional to higher powers of the laser frequency for hydrogenic atoms. The new analytical expressions for asymptotic ionization rates (which become accurate in the quasistatic limit) contain no summations over multiphoton contributions. For very low laser frequencies (optical or infrared), these expressions usually remain with an order-of-magnitude agreement with the velocity gauge strong-field approximation.

  4. Comparisons between a gas-phase model of silane chemical vapor deposition and laser-diagnostic measurements

    International Nuclear Information System (INIS)

    Theoretical modeling and experimental measurements have been used to study gas-phase chemistry in the chemical vapor deposition (CVD) of silicon from silane. Pulsed laser Raman spectroscopy was used to obtain temperature profiles and to obtain absolute density profiles of silane during deposition at atmospheric and 6-Torr total pressures for temperatures ranging from 500 to 8000C. Laser-excited fluorescence was used to obtain relative density profiles of Si2 during deposition at 740 0C in helium with 0-12 Torr added hydrogen. These measurements are compared to predictions from the theoretical model of Coltrin, Kee, and Miller. The predictions agree qualitatively with experiment. These studies indicate that fluid mechanics and gas-phase chemical kinetics are important considerations in understanding the chemical vapor deposition process

  5. Organic, inorganic and total mercury determination in fish by chemical vapor generation with collection on a gold gauze and electrothermal atomic absorption spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    Duarte, Fabio Andrei; Bizzi, Cezar Augusto; Goldschmidt Antes, Fabiane; Dressler, Valderi Luiz [Departamento de Quimica, Universidade Federal de Santa Maria, 97105-900 Santa Maria, RS (Brazil); Flores, Erico Marlon de Moraes [Departamento de Quimica, Universidade Federal de Santa Maria, 97105-900 Santa Maria, RS (Brazil)], E-mail: flores@quimica.ufsm.br

    2009-06-15

    A method for organic, inorganic and total mercury determination in fish tissue has been developed using chemical vapor generation and collection of mercury vapor on a gold gauze inside a graphite tube and further atomization by electrothermal atomic absorption spectrometry. After drying and cryogenic grinding, potassium bromide and hydrochloric acid solution (1 mol L{sup - 1} KBr in 6 mol L{sup - 1} HCl) was added to the samples. After centrifugation, total mercury was determined in the supernatant. Organomercury compounds were selectively extracted from KBr solution using chloroform and the resultant solution was back extracted with 1% m/v L-cysteine. This solution was used for organic Hg determination. Inorganic Hg remaining in KBr solution was directly determined by chemical vapor generation electrothermal atomic absorption spectrometry. Mercury vapor generation from extracts was performed using 1 mol L{sup - 1} HCl and 2.5% m/v NaBH{sub 4} solutions and a batch chemical vapor generation system. Mercury vapor was collected on the gold gauze heated resistively at 80 deg. C and the atomization temperature was set at 650 deg. C. The selectivity of extraction was evaluated using liquid chromatography coupled to chemical vapor generation and determination by inductively coupled plasma mass spectrometry. The proposed method was applied for mercury analysis in shark, croaker and tuna fish tissues. Certified reference materials were used to check accuracy and the agreement was better than 95%. The characteristic mass was 60 pg and method limits of detection were 5, 1 and 1 ng g{sup - 1} for organic, inorganic and total mercury, respectively. With the proposed method it was possible to analyze up to 2, 2 and 6 samples per hour for organic, inorganic and total Hg determination, respectively.

  6. Helium in chirped laser fields as a time-asymmetric atomic switch

    Czech Academy of Sciences Publication Activity Database

    Kaprálová-Žďánská, Petra Ruth; Moiseyev, N.

    2014-01-01

    Roč. 141, č. 1 (2014), 014307. ISSN 0021-9606 R&D Projects: GA ČR GAP205/11/0571 Institutional support: RVO:61388955 Keywords : Atom lasers * Laser pulses * Helium Subject RIV: CF - Physical ; Theoretical Chemistry Impact factor: 2.952, year: 2014

  7. Regularly arranged indium islands on glass/molybdenum substrates upon femtosecond laser and physical vapor deposition processing

    Science.gov (United States)

    Ringleb, F.; Eylers, K.; Teubner, Th.; Boeck, T.; Symietz, C.; Bonse, J.; Andree, S.; Krüger, J.; Heidmann, B.; Schmid, M.; Lux-Steiner, M.

    2016-03-01

    A bottom-up approach is presented for the production of arrays of indium islands on a molybdenum layer on glass, which can serve as micro-sized precursors for indium compounds such as copper-indium-gallium-diselenide used in photovoltaics. Femtosecond laser ablation of glass and a subsequent deposition of a molybdenum film or direct laser processing of the molybdenum film both allow the preferential nucleation and growth of indium islands at the predefined locations in a following indium-based physical vapor deposition (PVD) process. A proper choice of laser and deposition parameters ensures the controlled growth of indium islands exclusively at the laser ablated spots. Based on a statistical analysis, these results are compared to the non-structured molybdenum surface, leading to randomly grown indium islands after PVD.

  8. Model calculation of the characteristic mass for convective and diffusive vapor transport in graphite furnace atomic absorption spectrometry

    International Nuclear Information System (INIS)

    A combination of former convective–diffusive vapor-transport models is described to extend the calculation scheme for sensitivity (characteristic mass — m0) in graphite furnace atomic absorption spectrometry (GFAAS). This approach encompasses the influence of forced convection of the internal furnace gas (mini-flow) combined with concentration diffusion of the analyte atoms on the residence time in a spatially isothermal furnace, i.e., the standard design of the transversely heated graphite atomizer (THGA). A couple of relationships for the diffusional and convectional residence times were studied and compared, including in factors accounting for the effects of the sample/platform dimension and the dosing hole. These model approaches were subsequently applied for the particular cases of Ag, As, Cd, Co, Cr, Cu, Fe, Hg, Mg, Mn, Mo, Ni, Pb, Sb, Se, Sn, V and Zn analytes. For the verification of the accuracy of the calculations, the experimental m0 values were determined with the application of a standard THGA furnace, operating either under stopped, or mini-flow (50 cm3 min−1) of the internal sheath gas during atomization. The theoretical and experimental ratios of m0(mini-flow)-to-m0(stop-flow) were closely similar for each study analyte. Likewise, the calculated m0 data gave a fairly good agreement with the corresponding experimental m0 values for stopped and mini-flow conditions, i.e., it ranged between 0.62 and 1.8 with an average of 1.05 ± 0.27. This indicates the usability of the current model calculations for checking the operation of a given GFAAS instrument and the applied methodology. - Highlights: • A calculation scheme for convective–diffusive vapor loss in GFAAS is described. • Residence time (τ) formulas were compared for sensitivity (m0) in a THGA furnace. • Effects of the sample/platform dimension and dosing hole on τ were assessed. • Theoretical m0 of 18 analytes were calculated for stopped & mini furnace gas flows. • Experimental

  9. Model calculation of the characteristic mass for convective and diffusive vapor transport in graphite furnace atomic absorption spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    Bencs, László, E-mail: bencs.laszlo@wigner.mta.hu [Institute for Solid State Physics and Optics, Wigner Research Centre for Physics, Hungarian Academy of Sciences, P.O. Box 49, H-1525 Budapest (Hungary); Laczai, Nikoletta [Institute for Solid State Physics and Optics, Wigner Research Centre for Physics, Hungarian Academy of Sciences, P.O. Box 49, H-1525 Budapest (Hungary); Ajtony, Zsolt [Institute of Food Science, University of West Hungary, H-9200 Mosonmagyaróvár, Lucsony utca 15–17 (Hungary)

    2015-07-01

    A combination of former convective–diffusive vapor-transport models is described to extend the calculation scheme for sensitivity (characteristic mass — m{sub 0}) in graphite furnace atomic absorption spectrometry (GFAAS). This approach encompasses the influence of forced convection of the internal furnace gas (mini-flow) combined with concentration diffusion of the analyte atoms on the residence time in a spatially isothermal furnace, i.e., the standard design of the transversely heated graphite atomizer (THGA). A couple of relationships for the diffusional and convectional residence times were studied and compared, including in factors accounting for the effects of the sample/platform dimension and the dosing hole. These model approaches were subsequently applied for the particular cases of Ag, As, Cd, Co, Cr, Cu, Fe, Hg, Mg, Mn, Mo, Ni, Pb, Sb, Se, Sn, V and Zn analytes. For the verification of the accuracy of the calculations, the experimental m{sub 0} values were determined with the application of a standard THGA furnace, operating either under stopped, or mini-flow (50 cm{sup 3} min{sup −1}) of the internal sheath gas during atomization. The theoretical and experimental ratios of m{sub 0}(mini-flow)-to-m{sub 0}(stop-flow) were closely similar for each study analyte. Likewise, the calculated m{sub 0} data gave a fairly good agreement with the corresponding experimental m{sub 0} values for stopped and mini-flow conditions, i.e., it ranged between 0.62 and 1.8 with an average of 1.05 ± 0.27. This indicates the usability of the current model calculations for checking the operation of a given GFAAS instrument and the applied methodology. - Highlights: • A calculation scheme for convective–diffusive vapor loss in GFAAS is described. • Residence time (τ) formulas were compared for sensitivity (m{sub 0}) in a THGA furnace. • Effects of the sample/platform dimension and dosing hole on τ were assessed. • Theoretical m{sub 0} of 18 analytes were

  10. Laser-drilled micro-hole arrays on polyurethane synthetic leather for improvement of water vapor permeability

    Science.gov (United States)

    Wu, Y.; Wang, A. H.; Zheng, R. R.; Tang, H. Q.; Qi, X. Y.; Ye, B.

    2014-06-01

    Three kinds of lasers at 1064, 532 and 355 nm wavelengths respectively were adopted to construct micro-hole arrays on polyurethane (PU) synthetic leather with an aim to improve water vapor permeability (WVP) of PU synthetic leather. The morphology of the laser-drilled micro-holes was observed to optimize laser parameters. The WVP and slit tear resistance of the laser-drilled leather were measured. Results show that the optimized pulse energy for the 1064, 532 and 355 nm lasers are 0.8, 1.1 and 0.26 mJ, respectively. The diameters of the micro-holes drilled with the optimized laser pulse energy were about 20, 15 and 10 μm, respectively. The depths of the micro-holes drilled with the optimized pulse energy were about 21, 60 and 69 μm, respectively. Compared with the untreated samples, the highest WVP growth ratio was 38.4%, 46.8% and 53.5% achieved by the 1064, 532 and 355 nm lasers, respectively. And the highest decreasing ratio of slit tear resistance was 11.1%, 14.8%, and 22.5% treated by the 1064, 532 and 355 nm lasers, respectively. Analysis of the interaction mechanism between laser beams at three kinds of laser wavelengths and the PU synthetic leather revealed that laser micro-drilling at 355 nm wavelength displayed both photochemical ablation and photothermal ablation, while laser micro-drilling at 1064 and 532 nm wavelengths leaded to photothermal ablation only.

  11. Laser-drilled micro-hole arrays on polyurethane synthetic leather for improvement of water vapor permeability

    International Nuclear Information System (INIS)

    Three kinds of lasers at 1064, 532 and 355 nm wavelengths respectively were adopted to construct micro-hole arrays on polyurethane (PU) synthetic leather with an aim to improve water vapor permeability (WVP) of PU synthetic leather. The morphology of the laser-drilled micro-holes was observed to optimize laser parameters. The WVP and slit tear resistance of the laser-drilled leather were measured. Results show that the optimized pulse energy for the 1064, 532 and 355 nm lasers are 0.8, 1.1 and 0.26 mJ, respectively. The diameters of the micro-holes drilled with the optimized laser pulse energy were about 20, 15 and 10 μm, respectively. The depths of the micro-holes drilled with the optimized pulse energy were about 21, 60 and 69 μm, respectively. Compared with the untreated samples, the highest WVP growth ratio was 38.4%, 46.8% and 53.5% achieved by the 1064, 532 and 355 nm lasers, respectively. And the highest decreasing ratio of slit tear resistance was 11.1%, 14.8%, and 22.5% treated by the 1064, 532 and 355 nm lasers, respectively. Analysis of the interaction mechanism between laser beams at three kinds of laser wavelengths and the PU synthetic leather revealed that laser micro-drilling at 355 nm wavelength displayed both photochemical ablation and photothermal ablation, while laser micro-drilling at 1064 and 532 nm wavelengths leaded to photothermal ablation only.

  12. Mapping of laser diode radiation intensity by atomic-force microscopy

    Science.gov (United States)

    Alekseev, P. A.; Dunaevskii, M. S.; Slipchenko, S. O.; Podoskin, A. A.; Tarasov, I. S.

    2015-09-01

    The distribution of the intensity of laser diode radiation has been studied using an original method based on atomic-force microscopy (AFM). It is shown that the laser radiation intensity in both the near field and transition zone of a high-power semiconductor laser under room-temperature conditions can be mapped by AFM at a subwavelength resolution. The obtained patterns of radiation intensity distribution agree with the data of modeling and the results of near-field optical microscopy measurements.

  13. Numerical simulation of transient, incongruent vaporization induced by high power laser

    Energy Technology Data Exchange (ETDEWEB)

    Tsai, C.H.

    1981-01-01

    A mathematical model and numerical calculations were developed to solve the heat and mass transfer problems specifically for uranum oxide subject to laser irradiation. It can easily be modified for other heat sources or/and other materials. In the uranium-oxygen system, oxygen is the preferentially vaporizing component, and as a result of the finite mobility of oxygen in the solid, an oxygen deficiency is set up near the surface. Because of the bivariant behavior of uranium oxide, the heat transfer problem and the oxygen diffusion problem are coupled and a numerical method of simultaneously solving the two boundary value problems is studied. The temperature dependence of the thermal properties and oxygen diffusivity, as well as the highly ablative effect on the surface, leads to considerable non-linearities in both the governing differential equations and the boundary conditions. Based on the earlier work done in this laboratory by Olstad and Olander on Iron and on Zirconium hydride, the generality of the problem is expanded and the efficiency of the numerical scheme is improved. The finite difference method, along with some advanced numerical techniques, is found to be an efficient way to solve this problem.

  14. Field-deployable diode-laser-based differential absorption lidar (DIAL) for profiling water vapor

    Science.gov (United States)

    Spuler, S. M.; Repasky, K. S.; Morley, B.; Moen, D.; Hayman, M.; Nehrir, A. R.

    2015-03-01

    A field-deployable water vapor profiling instrument that builds on the foundation of the preceding generations of diode-laser-based differential absorption lidar (DIAL) laboratory prototypes was constructed and tested. Significant advances are discussed, including a unique shared telescope design that allows expansion of the outgoing beam for eye-safe operation with optomechanical and thermal stability; multistage optical filtering enabling measurement during daytime bright-cloud conditions; rapid spectral switching between the online and offline wavelengths enabling measurements during changing atmospheric conditions; and enhanced performance at lower ranges by the introduction of a new filter design and the addition of a wide field-of-view channel. Performance modeling, testing, and intercomparisons are performed and discussed. In general, the instrument has a 150 m range resolution with a 10 min temporal resolution; 1 min temporal resolution in the lowest 2 km of the atmosphere is demonstrated. The instrument is shown capable of autonomous long-term field operation - 50 days with a > 95% uptime - under a broad set of atmospheric conditions and potentially forms the basis for a ground-based network of eye-safe autonomous instruments needed for the atmospheric sciences research and forecasting communities.

  15. Field deployable diode-laser-based differential absorption lidar (DIAL) for profiling water vapor

    Science.gov (United States)

    Spuler, S. M.; Repasky, K. S.; Morley, B.; Moen, D.; Hayman, M.; Nehrir, A. R.

    2014-11-01

    A field deployable water vapor profiling instrument that builds on the foundation of the preceding generations of diode-laser-based differential absorption lidar (DIAL) laboratory prototypes has been constructed and tested. Significant advances are discussed, including: a unique shared telescope design that allows expansion of the outgoing beam for eye-safe operation with opto-mechanical and thermal stability, multi-stage optical filtering enabling measurement during daytime bright-cloud conditions, rapid spectral switching between the online and offline wavelengths enabling measurements during changing atmospheric conditions, and enhanced performance at lower ranges by the introduction of a new filter design and the addition of a wide field-of-view channel. Performance modeling, testing and intercomparisons have been performed and are discussed. In general, the instrument has 150 m range resolution with 10 min temporal resolution - 1 min temporal resolution in the lowest 2 km of the atmosphere is demonstrated. The instrument was shown capable of autonomous long term field operation - 50 days with a >95% uptime - under a broad set of atmospheric conditions and potentially forms the basis for a ground-based network of eye-safe autonomous instruments needed for the atmospheric sciences research and forecasting communities.

  16. Numerical simulation of transient, incongruent vaporization induced by high power laser

    International Nuclear Information System (INIS)

    A mathematical model and numerical calculations were developed to solve the heat and mass transfer problems specifically for uranum oxide subject to laser irradiation. It can easily be modified for other heat sources or/and other materials. In the uranium-oxygen system, oxygen is the preferentially vaporizing component, and as a result of the finite mobility of oxygen in the solid, an oxygen deficiency is set up near the surface. Because of the bivariant behavior of uranium oxide, the heat transfer problem and the oxygen diffusion problem are coupled and a numerical method of simultaneously solving the two boundary value problems is studied. The temperature dependence of the thermal properties and oxygen diffusivity, as well as the highly ablative effect on the surface, leads to considerable non-linearities in both the governing differential equations and the boundary conditions. Based on the earlier work done in this laboratory by Olstad and Olander on Iron and on Zirconium hydride, the generality of the problem is expanded and the efficiency of the numerical scheme is improved. The finite difference method, along with some advanced numerical techniques, is found to be an efficient way to solve this problem

  17. Monomolecular hydrogen elimination in C2H5OH vapor produced by CO2 IR laser pulses

    International Nuclear Information System (INIS)

    The authors examine the scope for the formation of acetaldehyde as a result of ethanol vapor photolysis by infrared multiphoton excitation and consequent isomerization via a series of probable reaction channels. The infrared source is a carbon dioxide laser. To estimate the relative probabilities of the channels they perform quantum-chemical calculations by the MINDO/3 method and vary all the independent degrees of freedom

  18. Atmospheric remote sensing of water vapor, HCl and CH4 using a continuously tunable Co:MgF2 laser

    Science.gov (United States)

    Menyuk, Norman; Killinger, Dennis K.

    1987-01-01

    A differential-absorption lidar system has been developed which uses a continuously tunable (1.5-2.3 micron) cobalt-doped magnesium fluoride laser as the radiation source. Preliminary atmospheric measurements of water vapor, HCl, and CH4 have been made with this system, including both path-averaged and ranged-resolved DIAL measurements at ranges up to 6 and 3 km, respectively.

  19. A scheme for the generation of two-mode atomic laser

    Institute of Scientific and Technical Information of China (English)

    Chunjia Huang(黄春佳); Ming Zhou(周明); Kewei Mo(莫克威)

    2003-01-01

    The quantum dynamic behavior of the system composed of V-type three-level atomic Bose-Einstein condensate (BEC) interacting with two-mode coherent light field has been studied. The results show that the atoms of V-type three-level atomic BEC, which are excited to higher-level states under the action of light field, still keep their properties of coherent states. It demonstrates theoretically that two-mode atomic laser may be prepared by V-type three-level atomic BEC.

  20. Model calculation of the characteristic mass for convective and diffusive vapor transport in graphite furnace atomic absorption spectrometry

    Science.gov (United States)

    Bencs, László; Laczai, Nikoletta; Ajtony, Zsolt

    2015-07-01

    A combination of former convective-diffusive vapor-transport models is described to extend the calculation scheme for sensitivity (characteristic mass - m0) in graphite furnace atomic absorption spectrometry (GFAAS). This approach encompasses the influence of forced convection of the internal furnace gas (mini-flow) combined with concentration diffusion of the analyte atoms on the residence time in a spatially isothermal furnace, i.e., the standard design of the transversely heated graphite atomizer (THGA). A couple of relationships for the diffusional and convectional residence times were studied and compared, including in factors accounting for the effects of the sample/platform dimension and the dosing hole. These model approaches were subsequently applied for the particular cases of Ag, As, Cd, Co, Cr, Cu, Fe, Hg, Mg, Mn, Mo, Ni, Pb, Sb, Se, Sn, V and Zn analytes. For the verification of the accuracy of the calculations, the experimental m0 values were determined with the application of a standard THGA furnace, operating either under stopped, or mini-flow (50 cm3 min- 1) of the internal sheath gas during atomization. The theoretical and experimental ratios of m0(mini-flow)-to-m0(stop-flow) were closely similar for each study analyte. Likewise, the calculated m0 data gave a fairly good agreement with the corresponding experimental m0 values for stopped and mini-flow conditions, i.e., it ranged between 0.62 and 1.8 with an average of 1.05 ± 0.27. This indicates the usability of the current model calculations for checking the operation of a given GFAAS instrument and the applied methodology.

  1. Enhancement of Efficiency of XUV Generation in Atomic Gases Irradiated by Intense Laser Fields

    Science.gov (United States)

    Andreev, A. V.; Stremoukhov, S. Y.; Shoutova, O. A.

    We present the results of the theoretical study of the high-order harmonic generation (HHG) in atomic gases. It is shown that the photoemission spectra exhibit unusual behavior when the laser field strength approaches near-atomic values. In subatomic field strength the cut-off frequency increases linearly with laser pulse intensity. However, when the field strength approaches near-atomic region firstly cut-off frequency slows down and then saturates. To interpret such kind of photoemission spectrum behavior we have proposed the light-atom interaction theory based on the use of eigenfunctions of boundary value problem for "an atom in the external field" instead of the traditional basis of the "free atom" eigenfunctions.

  2. Atomic force microscopy studies of homoepitaxial GaN layers grown on GaN template by laser MBE

    Science.gov (United States)

    Choudhary, B. S.; Singh, A.; Tanwar, S.; Tyagi, P. K.; Kumar, M. Senthil; Kushvaha, S. S.

    2016-04-01

    We have grown homoepitaxial GaN films on metal organic chemical vapor deposition (MOCVD) grown 3.5 µm thick GaN on sapphire (0001) substrate (GaN template) using an ultra-high vacuum (UHV) laser assisted molecular beam epitaxy (LMBE) system. The GaN films were grown by laser ablating a polycrystalline solid GaN target in the presence of active r.f. nitrogen plasma. The influence of laser repetition rates (10-30 Hz) on the surface morphology of homoepitaxial GaN layers have been studied using atomic force microscopy. It was found that GaN layer grown at 10 Hz shows a smooth surface with uniform grain size compared to the rough surface with irregular shape grains obtained at 30 Hz. The variation of surface roughness of the homoepitaxial GaN layer with and without wet chemical etching has been also studied and it was observed that the roughness of the film decreased after wet etching due to the curved structure/rough surface.

  3. Single-atom detection of ytterbium by selective laser excitation field ionization from Rydberg states

    International Nuclear Information System (INIS)

    Detection of single atoms Yb has been achieved using the method of electric-field ionization from the high-lying Rydberg states. Atoms of Yb in a beam were excited in three steps to a 17-p state by radiation of three pulsed dye lasers. The statistics of an atom's appearance in the interaction volume have been studied in the single-ion counting regime at low beam density

  4. Velocity distribution measurements in atomic beams generated using laser induced back-ablation

    CERN Document Server

    Denning, A; Lee, S; Ammonson, M; Bergeson, S D

    2008-01-01

    We present measurements of the velocity distribution of calcium atoms in an atomic beam generated using a dual-stage laser back-ablation apparatus. Distributions are measured using a velocity selective Doppler time-of-flight technique. They are Boltzmann-like with rms velocities corresponding to temperatures above the melting point for calcium. Contrary to a recent report in the literature, this method does not generate a sub-thermal atomic beam.

  5. Laser cooling of rubidium atoms in a magneto-optical trap

    OpenAIRE

    Hopkins, Stephen Anthony

    1996-01-01

    This thesis describes theoretical and experimental work concerning radiation forces on atoms, with particular reference to rubidium atoms confined in a magneto-optical trap. After a short history of the field of laser cooling, a review of the semiclassical theory of mechanical interactions between two-level atoms and electromagnetic radiation is given. Different formulations of the semiclassical theory are discussed, including a new formulation in terms of momentum transfer amongst the pl...

  6. Design of a laser neutral atom source for a collective accelerator

    International Nuclear Information System (INIS)

    Possible schemes are considered for storing and accelerating ions in electron rings using the collective heavy-ion accelerator (CHIA) at the Joint Institute for Nuclear Studies at Dubna. It is shown that the system can be supplied with ions by injecting a pulsed beam of atoms from a laser source into the electron ring. Tests of the laser source reveal that atomic beams of various elements can be produced which are well suited for use with the accelerator. The design and operation of some laser sources are discussed

  7. Generation of cold low divergent atomic beam of indium by laser ablation

    International Nuclear Information System (INIS)

    The formation of low-energy (below 100 m/s), low divergence (without any collimation optics) pulsed indium atomic beam via ablation of thin film by direct illumination (unfocused) from the rear side with second harmonic of Q-switched Nd:YAG laser under high vacuum (∼10-5 Torr) is reported. Angular divergence of an ablated indium beam was measured for the different laser powers. Axial atomic and ionic velocities were studied as a function of laser energy per pulse using a beam deflection setup

  8. Lasers as a Bridge between Atomic and Nuclear Physics

    OpenAIRE

    Matinyan, Sergei G.

    1997-01-01

    This paper reviews the application of optical and UV laser radiation to several topics in low-energy nuclear physics. We consider the laser-induced nuclear anti-Stokes transitions, the laser-assisted and the laser-induced internal conversion, and the Electron Bridge and Inverse Electron Bridge mechanisms as tools for deexciting and exciting of low-lying nuclear isomeric states. A study of the anomalous, by low-lying, nuclear isomeric states (on an example of the $^{229}$Th nucleus) is present...

  9. Efficient sub-Doppler transverse laser cooling of an indium atomic beam

    Energy Technology Data Exchange (ETDEWEB)

    Kim, Jae-Ihn

    2009-07-23

    Laser cooled atomic gases and atomic beams are widely studied samples in experimental research in atomic and optical physics. For the application of ultra cold gases as model systems for e.g. quantum many particle systems, the atomic species is not very important. Thus this field is dominated by alkaline, earthalkaline elements which are easily accessible with conventional laser sources and have convenient closed cooling transition. On the other hand, laser cooled atoms may also be interesting for technological applications, for instance for the creation of novel materials by atomic nanofabrication (ANF). There it will be important to use technologically relevant materials. As an example, using group III atoms of the periodical table in ANF may open a route to generate fully 3D structured composite materials. The minimal requirement in such an ANF experiment is the collimation of an atomic beam which is accessible by one dimensional laser cooling. In this dissertation, I describe transverse laser cooling of an Indium atomic beam. For efficient laser cooling on a cycling transition, I have built a tunable, continuous-wave coherent ultraviolet source at 326 nm based on frequency tripling. For this purpose, two independent high power Yb-doped fiber amplifiers for the generation of the fundamental radiation at {lambda}{sub {omega}} = 977 nm have been constructed. I have observed sub-Doppler transverse laser cooling of an Indium atomic beam on a cycling transition of In by introducing a polarization gradient in the linear-perpendicular-linear configuration. The transverse velocity spread of a laser-cooled In atomic beam at full width at half maximum was achieved to be 13.5{+-}3.8 cm/s yielding a full divergence of only 0.48 {+-} 0.13 mrad. In addition, nonlinear spectroscopy of a 3-level, {lambda}-type level system driven by a pump and a probe beam has been investigated in order to understand the absorption line shapes used as a frequency reference in a previous two

  10. Laser diagnostics of the energy spectrum of Rydberg states of the lithium-7 atom

    Energy Technology Data Exchange (ETDEWEB)

    Zelener, B. B., E-mail: bobozel@mail.ru; Saakyan, S. A.; Sautenkov, V. A.; Manykin, E. A.; Zelener, B. V.; Fortov, V. E. [Russian Academy of Sciences, Joint Institute for High Temperatures (Russian Federation)

    2015-12-15

    The spectra of excited lithium-7 atoms prepared in a magneto-optical trap are studied using a UV laser. The laser diagnostics of the energy of Rydberg atoms is developed based on measurements of the change in resonance fluorescence intensity of ultracold atoms as the exciting UV radiation frequency passes through the Rydberg transition frequency. The energies of various nS configurations are obtained in a broad range of the principal quantum number n from 38 to 165. The values of the quantum defect and ionization energy obtained in experiments and predicted theoretically are discussed.

  11. Theoretical study on isotope separation of an ytterbium atomic beam by laser deflection

    International Nuclear Information System (INIS)

    Isotope separation by laser deflecting an atomic beam is analyzed theoretically. Interacting with a tilted one-dimensional optical molasses, an ytterbium atomic beam is split into multi-beams with different isotopes like 172Yb,173Yb, and 174Yb. By using the numerical calculation, the dependences of the splitting angle on the molasses laser intensity and detuning are studied, and the optimal parameters for the isotope separation are also investigated. Furthermore, the isotope separation efficiency and purity are estimated. Finally a new scheme for the efficient isotope separation is proposed. These findings will give a guideline for simply obtaining pure isotopes of various elements. (atomic and molecular physics)

  12. Efficient sub-Doppler transverse laser cooling of an indium atomic beam

    International Nuclear Information System (INIS)

    Laser cooled atomic gases and atomic beams are widely studied samples in experimental research in atomic and optical physics. For the application of ultra cold gases as model systems for e.g. quantum many particle systems, the atomic species is not very important. Thus this field is dominated by alkaline, earthalkaline elements which are easily accessible with conventional laser sources and have convenient closed cooling transition. On the other hand, laser cooled atoms may also be interesting for technological applications, for instance for the creation of novel materials by atomic nanofabrication (ANF). There it will be important to use technologically relevant materials. As an example, using group III atoms of the periodical table in ANF may open a route to generate fully 3D structured composite materials. The minimal requirement in such an ANF experiment is the collimation of an atomic beam which is accessible by one dimensional laser cooling. In this dissertation, I describe transverse laser cooling of an Indium atomic beam. For efficient laser cooling on a cycling transition, I have built a tunable, continuous-wave coherent ultraviolet source at 326 nm based on frequency tripling. For this purpose, two independent high power Yb-doped fiber amplifiers for the generation of the fundamental radiation at λω = 977 nm have been constructed. I have observed sub-Doppler transverse laser cooling of an Indium atomic beam on a cycling transition of In by introducing a polarization gradient in the linear-perpendicular-linear configuration. The transverse velocity spread of a laser-cooled In atomic beam at full width at half maximum was achieved to be 13.5±3.8 cm/s yielding a full divergence of only 0.48 ± 0.13 mrad. In addition, nonlinear spectroscopy of a 3-level, Λ-type level system driven by a pump and a probe beam has been investigated in order to understand the absorption line shapes used as a frequency reference in a previous two-color spectroscopy experiment

  13. Interference Dynamics of Hydrogen Atoms in High-Frequency Dichromatic Laser Fields

    Institute of Scientific and Technical Information of China (English)

    程太旺; 李晓峰; 傅盘铭; 陈式刚

    2002-01-01

    We investigate the ionization and high-order harmonic generation of a hydrogen atom in high-frequency (several atomic units) super strong (up to several tens of atomic units) dichromatic laser fields. An effective iterative method in the framework of high-frequency Floquet theory is used in the calculations. We have considered two kinds of dichromatic laser field, i.e. 1ω - 2ω and lω - 3ω. We find that, in both the cases, the ionization and high-order harmonic generation show evident dependence on the relative phase and strength of the additional harmonic field. The dynamical origin of these interference effects is also discussed.

  14. Non-additivity in laser-illuminated many-atom systems

    CERN Document Server

    Shahmoon, Ephraim; Kurizki, Gershon

    2013-01-01

    We show that atoms subject to laser radiation may form a non-additive many-body system on account of their long-range interactions, when the atoms are trapped in the vicinity of a fiber with Bragg grating. When the laser frequency is inside the grating's bandgap but very close to its edge, we find that the range and strength of the laser-induced interaction becomes substantially enhanced, due to the large density of states near the edge, while the competing process of scattering to the fiber is inhibited. The dynamics of this system conforms to a prominent model of statistical physics which exhibits slow relaxation. This suggests the possibility of using laser-illuminated atoms to study the characteristics of non-additive systems.

  15. Effects of laser radiation field on energies of hydrogen atom in plasmas

    International Nuclear Information System (INIS)

    In this study, for the first time, the Schrödinger equation with more general exponential cosine screened Coulomb (MGECSC) potential is solved numerically in the presence of laser radiation field within the Ehlotzky approximation using the asymptotic iteration method. The MGECSC potential includes four different potential forms in consideration of different sets of the parameters in the potential. By applying laser field, the total interaction potential of hydrogen atom embedded in plasmas converts to double well-type potential. The plasma screening effects under the influence of laser field as well as confinement effects of laser field on hydrogen atom in Debye and quantum plasmas are investigated by solving the Schrödinger equation with the laser-dressed MGECSC potential. It is resulted that since applying a monochromatic laser field on hydrogen atom embedded in a Debye and quantum plasma causes to shift in the profile of the total interaction potential, the confinement effects of laser field on hydrogen atom in plasmas modeled by the MGECSC potential change localizations of energy states

  16. On-line preconcentration and determination of mercury in biological and environmental samples by cold vapor-atomic absorption spectrometry

    International Nuclear Information System (INIS)

    An on-line procedure for the determination of traces of total mercury in environmental and biological samples is described. The present methodology combines cold vapor generation associated to atomic absorption spectrometry (CV-AAS) with preconcentration of the analyte on a minicolumn packed with activated carbon. The retained analyte was quantitatively eluted from the minicolumn with nitric acid. After that, volatile specie of mercury was generated by merging the acidified sample and sodium tetrahydroborate(III) in a continuous flow system. The gaseous analyte was subsequently introduced via a stream of Ar carrier into the atomizer device. Optimizations of both, preconcentration and mercury volatile specie generation variables were carried out using two level full factorial design (23) with 3 replicates of the central point. Considering a sample consumption of 25 mL, an enrichment factor of 13-fold was obtained. The detection limit (3σ) was 10 ng L-1 and the precision (relative standard deviation) was 3.1% (n = 10) at the 5 μg L-1 level. The calibration curve using the preconcentration system for mercury was linear with a correlation coefficient of 0.9995 at levels near the detection limit up to at least 1000 μg L-1. Satisfactory results were obtained for the analysis of mercury in tap water and hair samples

  17. Ultra-trace determination of methylmercuy in seafood by atomic fluorescence spectrometry coupled with electrochemical cold vapor generation.

    Science.gov (United States)

    Zu, Wenchuan; Wang, Zhenghao

    2016-03-01

    A homemade electrochemical flow cell was adopted for the determination of methylmercury. The cold vapor of mercury atoms was generated from the surface of glassycarbon cathode through the method of electrolytic reduction and detected by atomic fluorescence spectroscopy subsequently. The operating conditions were optimized with 2 ng mL(-1) methylmercury standard solution. The caliberation curve was favorably linear when the concentrations of standard HgCH3(+) solutions were in the range of 0.2-5 ng mL(-1)(as Hg). Under the optimized conditions, the limit of detection (LOD) for methylmercury was 1.88×10(-3)ng mL(-1) and the precision evaluated by relative standard deviation was 2.0% for six times 2 ng mL(-1) standard solution replicates. The terminal analytical results of seafood samples, available from local market, showed that the methylmercury content ranged within 3.7-45.8 ng g(-1). The recoveries for methylmercury spiked samples were found to be in the range of 87.6-103.6% and the relative standard deviations below 5% (n=6) were acquired, which showed this method was feasible for real sample analysis. PMID:26615576

  18. Mechanisms of infrared-laser-assisted atomic ionization by attosecond pulses

    International Nuclear Information System (INIS)

    We propose a mechanism to understand the infrared (IR) laser assisted atomic ionization by attosecond pulses (AP). Atomic structures in an IR laser field are described by Floquet states and atoms can be ionized to a Floquet state by a single AP through different Floquet components. The interference of ionization through different Floquet components results in the oscillation of the ionization yield as a function of the arriving time of the AP. The proposed mechanism explains the recent experimental observations [Johnsson et al., Phys. Rev. Lett. 99, 233001 (2007)]. Furthermore, we find that, for a specified photoelectron energy, the ionization yield always oscillates as a function of the relative phase between the AP and the IR laser for both He and Ar atoms.

  19. Laser-excitation atomic fluorescence spectroscopy in a helium microwave-induced plasma

    Science.gov (United States)

    Schroeder, Timothy S.

    The focus of this dissertation is to report the first documented coupling of helium microwave induced plasmas (MIPs) to laser excitation atomic fluorescence spectroscopy. The ability to effectively produce intense atomic emission from both metal and nonmetal analytes gives helium microwave induced plasmas a greater flexibility than the more commonly utilized argon inductively coupled plasma (ICP). Originally designed as an element selective detector for non-aqueous chromatography applications at low applied powers (plasma has been applied to aqueous sample determinations at higher applied powers (>500 W). The helium MIP has been shown to be a very powerful analytical atomic spectroscopy tool. The development of the pulsed dye laser offered an improved method of excitation in the field of atomic fluorescence. The use of laser excitation for atomic fluorescence was a logical successor to the conventional excitation methods involving hollow cathode lamps and continuum sources. The highly intense, directional, and monochromatic nature of laser radiation results in an increased population of atomic species in excited electronic states where atomic fluorescence can occur. The application of laser excitation atomic fluorescence to the analysis of metals in a helium microwave induced plasma with ultrasonic sample nebulization was the initial focus of this work. Experimental conditions and results are included for the aqueous characterization of manganese, lead, thallium, and iron in the helium MIP- LEAFS system. These results are compared to previous laser excitation atomic fluorescence experimentation. The effect of matrix interferences on the analytical fluorescence signal was also investigated for each element. The advantage of helium MIPs over argon ICPs in the determination of nonmetals in solution indicates that the helium MIP is an excellent candidate for laser excitation atomic fluorescence experiments involving nonmetals such as chlorine, bromine, iodine, and

  20. NATO Advanced Study Institute on Laser Interactions with Atoms, Solids,and Plasmas

    CERN Document Server

    1994-01-01

    The aim of this NATO Advanced Study Institute was to bring together scientists and students working in the field of laser matter interactions in order to review and stimulate developmentoffundamental science with ultra-short pulse lasers. New techniques of pulse compression and colliding-pulse mode-locking have made possible the construction of lasers with pulse lengths in the femtosecond range. Such lasers are now in operation at several research laboratories in Europe and the United States. These laser facilities present a new and exciting research direction with both pure and applied science components. In this ASI the emphasis is on fundamental processes occurring in the interaction of short laser pulses with atoms, molecules, solids, and plasmas. In the case of laser-atom (molecule) interactions, high power lasers provide the first access to extreme high-intensity conditions above 10'8 Watts/em', a new frontier for nonlinear interaction of photons with atoms and molecules. New phenomena observed include ...

  1. ERDA characterization of CN films prepared by laser-induced chemical vapor deposition

    International Nuclear Information System (INIS)

    The development of new materials exhibiting useful mechanical, electronic or magnetic properties represents a central challenge of materials research. Among the wide array of important properties, hardness is a characteristic that may be possible to understand theoretically. It represents an ideal one to test our ability to design materials with predictable properties. Since the first theoretical predictions about the existence and outstanding properties of carbon nitride, extended experimental work was performed in order to obtain this material with precise stoichiometry and structure applying a wide variety of methods. Among others, laser techniques have reached good results in the formation of CNx layers. Elastic recoil detection analysis (ERDA) technique may be useful as a characterization method of thin films, especially to determine their stoichiometry and perform depth profiling. We performed the synthesis of thin CNx films on silicon wafers using a CW CO2 laser (∼80 Watt). The laser beam was directed perpendicularly to the substrate. The substrate was continuously flowed by a mixture of reactant gases (mainly, ethylene of different concentrations, as carbon donor, ammonia, as nitrogen donor and an oxidizing agent (N2O) which could accelerate molecular decomposition). By heating the substrate at temperatures of several hundred degrees, the CO2 laser radiation induces pyrolysis reactions at the surface and interface, promoting reactant decomposition and radical reactions whose end-products condense onto the solid surface under the form of an adhesive thin solid film. Composition and thickness of the CNx samples were measured by ERDA using an 80 MeV, 63Cu10+ beam provided by the Tandem Van de Graaff accelerator of IFIN-HH. The samples were tilted to an angle of 15 angle with regard to the beam direction. A ΔE(gas)-E(solid) compact detector telescope was placed at 30 angle with respect to the beam. The measured ΔE-E spectrum and the energy spectra for C and

  2. Chemical reactions of excited nitrogen atoms for short wavelength chemical lasers. Final technical report

    Energy Technology Data Exchange (ETDEWEB)

    1989-12-15

    Accomplishments of this program include the following: (1) Scalable, chemical generation of oxygen atoms by reaction of fluorine atoms and water vapor. (2) Production of nitrogen atom densities of 1 {times} 10{sup 1}5 cm{sup {minus}3} with 5% electrical efficiency by injecting trace amounts of fluorine into microwave discharged nitrogen. (3) Production of cyanide radicals by reaction of high densities of N atoms with cyanogen. (4) Production of carbon atoms by reaction of nitrogen atoms with cyanogen or with fluorine atoms and hydrogen cyanide. (5) Confirmation that the reaction of carbon atoms and carbonyl sulfide produces CS(a{sup 3} {Pi}{sub r}), as predicted by conservation of electron spin and orbital angular momenta and as proposed by others under another SWCL program. (6) Production of cyanide radicals by injection of cyanogen halides into active nitrogen and use as spectroscopic calibration source. (7) Demonstration that sodium atoms react with cyanogen chloride, bromide and iodide and with cyanuric trifluoride to produce cyanide radicals. (8) Demonstration of the potential utility of the fluorine atom plus ammonia reaction system in the production of NF(b{sup l}{Sigma}{sup +}) via N({sup 2}D) + F{sub 2}.

  3. Laser Programs Highlight 1995

    Energy Technology Data Exchange (ETDEWEB)

    Jacobs, R.R.

    1997-01-31

    Our contributions to laser science and technology and corresponding applications range from concept to design of the National Ignition Facility, transfer of Atomic Vapor Laser Isotope Separation technology to the private sector, and from new initiatives in industry and defense to micro-optics for improving human vision.

  4. Multiphoton resonant ionization of hydrogen atom exposed to two-colour laser pulses

    Institute of Scientific and Technical Information of China (English)

    Wang Pei-Jie; Fang Yan

    2008-01-01

    This paper studies the multiphoton resonant ionization by two-colour laser pulses in the hydrogen atom by solving the time-dependent Schr(o)dinger equation.By fixing the parameters of fundamental laser field and scanning the frequency of second laser field,it finds that the ionization probability shows several resonance peaks and is also much larger than the linear superposition of probabilities by applying two lasers separately.The enhancement of the ionization happens when the system is resonantly pumped to the excited states by absorbing two or more colour photons non-sequentially.

  5. Chemical oxygen-iodine laser with instantaneous production of atomic iodine from gaseous reactants

    Czech Academy of Sciences Publication Activity Database

    Jirásek, Vít; Špalek, Otomar; Čenský, Miroslav; Kodymová, Jarmila; Jakubec, Ivo

    Bellingham: SPIE, 2006 - (Bohn, W.), 605307/1-605307/8. (Proceedings of SPIE. 6053). ISBN 0-8194-6326-4. ISSN 0277-786X. [International Conference on Lasers, Applications, and Technologies 2005: High Power Lasers and Applications. St. Petersburg (RU), 11.05.2005-15.05.2005] Grant ostatní: USAF EOARD(US) FA8655-02-M4040 Institutional research plan: CEZ:AV0Z10100523; CEZ:AV0Z40320502 Keywords : atomic iodine * supersonic mixing * chemical oxygen-iodine laser Subject RIV: BH - Optics, Masers, Lasers

  6. Design and Fabrication of a Chip-based Continuous-wave Atom Laser

    CERN Document Server

    Power, E P; Vanderelzen, B; Herrera-Fierro, P; Murphy, R; Yalisove, S M; Raithel, G

    2012-01-01

    We present a design for a continuous-wave (CW) atom laser on a chip and describe the process used to fabricate the device. Our design aims to integrate quadrupole magnetic guiding of ground state Rb atoms with continuous surface adsorption evaporative cooling to create a continuous Bose-Einstein condensate; out-coupled atoms from the condensate should realize a CW atom laser. We choose a geometry with three wires embedded in a spiral pattern in a silicon subtrate. The guide features an integrated solenoid to mitigate spin-flip losses and provide a tailored longitudinal magnetic field. Our design also includes multiple options for atom interferometry: accomodations are in place for laser-generated atom Fabry-Perot and Mach-Zehnder interferometers, and a pair of atomic beam X-splitters is incorporated for an all-magnetic atom Mach-Zehnder setup. We demonstrate the techniques necessary to fabricate our device using existing micro- and nano-scale fabrication equipment, and discuss future options for modified desi...

  7. Tomography of laser cooled atoms in MOT using Rydberg state excitation

    International Nuclear Information System (INIS)

    Full text: The position selective dimensional study of laser cooled atoms in Magneto-Optical Trap (MOT) is usually performed using optical detection. Nevertheless, many years ago a more precise method of imaging of atomic beams was developed using ionization of atoms and detection of produced electrons and ions using secondary electron multipliers. This technique demonstrates the possibility to detect a few atoms making it attractive for experiments with a small density of atoms. In the current paper we have performed an experiment directed to observe the difference in the space distribution of Rb atoms in MOT in the first exited state (5P) caused various selection (dark or bright) of the repumping transition. In the our experiment we produced a cold atomic cloud of 107 Rb atoms cooled using conventional MOT setup. After that atoms were optically exited to the Rydberg state using cascade transitions: 5S→5P→8S (decay)→ 6P→nS;nD (n ∼ 37). First excitation pulse (5P→8S) was performed by pulsed dye laser (Rodamine G6, 615 nm). Second, pulse of the Ti:Sa laser at 740 nm was applied to the transitions 6P→ nS;nD. Laser beams were focused to the trap and crossed under angle near 90 degree. The Rydberg atoms were detected using selective field ionization technique. The Ti:Sa laser beam was 1D scanned across the atomic cloud using a deffector based on galvanometer driven lens. The optical detection unit was controlled using a computer. It allows us to make position sensitive measurements of the Rydberg state excitation rate. Averaged data on counts of Rydberg atoms was used to determine population of the 5P state in separate parts of the atomic cloud. Experimental tomography data obtained for locking of the repumping laser to the bright or dark transition, show different 5P 1D profiles of the trap. Observed phenomena were in agreement with theoretical predictions and our previous results. This technique is a non-destructive method of measurement of exited state

  8. Laser Cooling without Repumping: A Magneto-Optical Trap for Erbium Atoms

    International Nuclear Information System (INIS)

    We report on a novel mechanism that allows for strong laser cooling of atoms that do not have a closed cycling transition. This mechanism is observed in a magneto-optical trap (MOT) for erbium, an atom with a very complex energy level structure with multiple pathways for optical-pumping losses. We observe surprisingly high trap populations of over 106 atoms and densities of over 1011 atoms cm-3, despite the many potential loss channels. A model based on recycling of metastable and ground state atoms held in the quadrupole magnetic field of the trap explains the high trap population, and agrees well with time-dependent measurements of MOT fluorescence. The demonstration of trapping of a rare-earth atom such as erbium opens a wide range of new possibilities for practical applications and fundamental studies with cold atoms

  9. Soft-Bake Purification of SWCNTs Produced by Pulsed Laser Vaporization

    Science.gov (United States)

    Yowell, Leonard; Nikolaev, Pavel; Gorelik, Olga; Allada, Rama Kumar; Sosa, Edward; Arepalli, Sivaram

    2013-01-01

    The "soft-bake" method is a simple and reliable initial purification step first proposed by researchers at Rice University for single-walled carbon nanotubes (SWCNT) produced by high-pressure carbon mon oxide disproportionation (HiPco). Soft-baking consists of annealing as-produced (raw) SWCNT, at low temperatures in humid air, in order to degrade the heavy graphitic shells that surround metal particle impurities. Once these shells are cracked open by the expansion and slow oxidation of the metal particles, the metal impurities can be digested through treatment with hydrochloric acid. The soft-baking of SWCNT produced by pulsed-laser vaporization (PLV) is not straightforward, because the larger average SWCNT diameters (.1.4 nm) and heavier graphitic shells surrounding metal particles call for increased temperatures during soft-bake. A part of the technology development focused on optimizing the temperature so that effective cracking of the graphitic shells is balanced with maintaining a reasonable yield, which was a critical aspect of this study. Once the ideal temperature was determined, a number of samples of raw SWCNT were purified using the soft-bake method. An important benefit to this process is the reduced time and effort required for soft-bake versus the standard purification route for SWCNT. The total time spent purifying samples by soft-bake is one week per batch, which equates to a factor of three reduction in the time required for purification as compared to the standard acid purification method. Reduction of the number of steps also appears to be an important factor in improving reproducibility of yield and purity of SWCNT, as small deviations are likely to get amplified over the course of a complicated multi-step purification process.

  10. Flux correction for closed-path laser spectrometers without internal water vapor measurements

    Science.gov (United States)

    Hiller, R. V.; Zellweger, C.; Knohl, A.; Eugster, W.

    2012-01-01

    Recently, instruments became available on the market that provide the possibility to perform eddy covariance flux measurements of CH4 and many other trace gases, including the traditional CO2 and H2O. Most of these instruments employ laser spectroscopy, where a cross-sensitivity to H2O is frequently observed leading to an increased dilution effect. Additionally, sorption processes at the intake tube walls modify and delay the observed H2O signal in closed-path systems more strongly than the signal of the sampled trace gas. Thereby, a phase shift between the trace gas and H2O fluctuations is introduced that dampens the H2O flux observed in the sampling cell. For instruments that do not provide direct H2O measurement in the sampling cell, transfer functions from externally measured H2O fluxes are needed to estimate the effect of H2O on trace gas flux measurements. The effects of cross-sensitivity and the damping are shown for an eddy covariance setup with the Fast Greenhouse Gas Analyzer (FGGA, Los Gatos Research Inc.) that measures CO2, CH4, and H2O fluxes. This instrument is technically identical with the Fast Methane Analyzer (FMA, Los Gatos Research Inc.) that does not measure H2O concentrations. Hence, we used measurements from a FGGA to derive a modified correction for the FMA accounting for dilution as well as phase shift effects in our instrumental setup. With our specific setup for eddy covariance flux measurements, the cross-sensitivity counteracts the damping effects, which compensate each other. Hence, the new correction only deviates very slightly from the traditional Webb, Pearman, and Leuning density correction, which is calculated from separate measurements of the atmospheric water vapor flux.

  11. Study of helium and beryllium atoms with strong and short laser field; Etude des atomes d'helium et de beryllium en champ laser intense et bref

    Energy Technology Data Exchange (ETDEWEB)

    Laulan, St

    2004-09-01

    We present a theoretical study of the interaction between a two-active electron atom and an intense (10{sup 14} to 10{sup 15} W/cm{sup 2}) and ultrashort (from a few 10{sup -15} to a few 10{sup -18} s) laser field. In the first part, we describe the current experimental techniques able to produce a coherent radiation of high power in the UV-XUV regime and with femtosecond time duration. A theoretical model of a laser pulse is defined with such characteristics. Then, we develop a numerical approach based on B-spline functions to describe the atomic structure of the two-active electron system. A spectral non perturbative method is proposed to solve the time dependent Schroedinger equation. We focalize our attention on the description of the atomic double continuum states. Finally, we expose results on the double ionization of helium and beryllium atoms with intense and short laser field. In particular, we present total cross section calculations and ejected electron energy distributions in the double continuum after one- and two-photon absorption. (author)

  12. Narrow spectral width laser diode for metastable argon atoms pumping

    Science.gov (United States)

    Gao, Jun; Li, Bin; Wang, Xinbing; Zuo, Duluo

    2016-03-01

    Diode laser pump source with narrow emitting spectrum for optically pumped metastable rare gas laser (OPRGL) of argon was achieved by employing a complex external cavity coupled with volume Bragg grating (VBG). A commercially available c-mount laser diode with rated power of 6 W was used and studied in both the free running mode and VBG external cavity. The maximum output power of 3.9 W with FWHM less than 25 pm and peak wavelength locked around 811.53 nm was obtained from the VBG external cavity laser diode. Precise control of VBG temperature enabled fine tuning of the emission wavelength over a range of 450 pm. Future researches on OPRGL of argon will benefit from it.

  13. Characterization of laser - induced plasmas by atomic emission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Diaz Pace, Diego M; Bertuccelli, Graciela; D' Angelo, Cristian A, E-mail: ddiaz@exa.unicen.edu.ar, E-mail: gbertucc@exa.unicen.edu.ar, E-mail: cdangelo@exa.unicen.edu.ar [Instituto de Fisica ' Arroyo Seco' , Facultad de Ciencias Exactas, U.N.C.P.B.A., Campus Universitario, Paraje Arroyo Seco, (B7000GHG) Tandil, Buenos Aires (Argentina)

    2011-01-01

    In this work, Laser-induced breakdown spectroscopy (LIBS) has been applied to characterization of plasmas generated in air at atmospheric pressure from a calcium hydroxide sample with a known concentration of Mg by using an infrared Nd:YAG laser. The influence of laser irradiance on plasma morphology and emission intensity was studied. Spatially-integrated intensities of Mg I-II lines along the line-of-sight were measured for different laser energies and delay times. The plasma temperature and the electron density were determined in each case by using and algorithm that calculates the optical thickness of the spectral lines and reproduces their experimental profiles in a framework of an homogeneous plasma in LTE that takes into account the effects of self-absorption. The results obtained showed the usefulness of this approach to provide additional information retrieved from the optical thickness of spectral lines for plasma characterization in LIBS experiments.

  14. High-order-harmonic generation from Rydberg atoms driven by plasmon-enhanced laser fields

    Science.gov (United States)

    Tikman, Y.; Yavuz, I.; Ciappina, M. F.; Chacón, A.; Altun, Z.; Lewenstein, M.

    2016-02-01

    We theoretically investigate high-order-harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should exceed a certain threshold in order to stimulate HHG when noble gas atoms in their ground state are used as an active medium. One way to enhance the coherent light coming from a conventional laser oscillator is to take advantage of the amplification obtained by the so-called surface plasmon polaritons, created when a low-intensity laser field is focused onto a metallic nanostructure. The main limitation of this scheme is the low damage threshold of the materials employed in the nanostructure engineering. In this work we propose the use of Rydberg atoms, driven by spatially inhomogeneous, plasmon-enhanced laser fields, for HHG. We exhaustively discuss the behavior and efficiency of these systems in the generation of coherent harmonic emission. Toward this aim we numerically solve the time-dependent Schrödinger equation for an atom, with an electron initially in a highly excited n th Rydberg state, located in the vicinity of a metallic nanostructure. In this zone the electric field changes spatially on scales relevant for the dynamics of the laser-ionized electron. We first use a one-dimensional model to investigate systematically the phenomena. We then employ a more realistic situation, in which the interaction of a plasmon-enhanced laser field with a three-dimensional hydrogen atom is modeled. We discuss the scaling of the relevant input parameters with the principal quantum number n of the Rydberg state in question and demonstrate that harmonic emission can be achieved from Rydberg atoms well below the damage threshold, thus without deterioration of the geometry and properties of the metallic nanostructure.

  15. Mathematical model of isotope-selective laser excitation of long-lived levels of atoms

    International Nuclear Information System (INIS)

    Method of laser isotope separation base on monophoton selective excitation of long-lived states of atoms could be classified as a new one. Taking zinc and rubidium as an example it is shown that long-lived excited states of atoms could effectively chemically react with a number of molecules, whereas basic states of atoms react weakly. In contrast to AVLIS the method is based on the use of one wavelength. This method does not require collimation of flow of atoms and electric extraction. The method uses Doppler contour property. This property resides in that frequency tuning increasing simultaneously from all the isotopes excitation selectivity rises

  16. Classical trajectory perspective of atomic ionization in strong laser fields. Semiclassical modeling

    International Nuclear Information System (INIS)

    Dealing with timely and interesting issues in strong laser physics. Illustrates complex strong field atomic ionization with the simple semiclassical model of classical trajectory perspective for the first time. Provides a theoretical model that can be used to account for recent experiments. The ionization of atoms and molecules in strong laser fields is an active field in modern physics and has versatile applications in such as attosecond physics, X-ray generation, inertial confined fusion (ICF), medical science and so on. Classical Trajectory Perspective of Atomic Ionization in Strong Laser Fields covers the basic concepts in this field and discusses many interesting topics using the semiclassical model of classical trajectory ensemble simulation, which is one of the most successful ionization models and has the advantages of a clear picture, feasible computing and accounting for many exquisite experiments quantitatively. The book also presents many applications of the model in such topics as the single ionization, double ionization, neutral atom acceleration and other timely issues in strong field physics, and delivers useful messages to readers with presenting the classical trajectory perspective on the strong field atomic ionization. The book is intended for graduate students and researchers in the field of laser physics, atom molecule physics and theoretical physics. Dr. Jie Liu is a professor of Institute of Applied Physics and Computational Mathematics, China and Peking University.

  17. Laser-induced photofragmentation of triethylaluminum: Modeling H-atom production

    Science.gov (United States)

    Brum, Jeffrey L.; Deshmukh, Subhash; Koplitz, Brent

    1990-12-01

    A rate-equation approach is presented that models H-atom formation during the pulsed laser photolysis of a triethyl metal compound, the specific case being triethylaluminum excited at 193 nm. An excimer laser initiates the chemistry under collisionless conditions, and H atoms are produced that are detected using two-photon (121.6+364.7 nm) ionization. Experimentally, the H-atom intensity is monitored as a function of photolysis laser power. Mechanistically, the primary photodissociation step is postulated to involve cleavage of the metal-carbon bond, thereby producing an ethyl radical. This species can then either: (1) form C2H4 and H directly; or (2) absorb an additional photon and produce an H-atom photofragment. The rate equations and their solutions allow one to calculate how H-atom production should vary as a function of photolysis laser power, and the interplay between the two H-atom production channels is calculated for various absorption cross sections and dissociation rates. A comparison with experimental power dependence data suggests that an overall one-photon dissociation process predominates under the experimental conditions actually used.

  18. Atomic force microscopy visualization of injuries in Enterococcus faecalis surface caused by Er,Cr:YSGG and diode lasers

    OpenAIRE

    López Jiménez, Lidia; Arnabat Domínguez, Josep; Viñas Ciordia, Miquel; Vinuesa Aumedes, Teresa

    2015-01-01

    Aim: To visualize by Atomic Force Microscopy the alterations induced on Enterococcus. faecalis surface after treatment with 2 types of laser: Erbium chromium:yttrium-scandium-gallium-garnet (Er,Cr:YSGG) laser and Diode laser. Material and Methods: Bacterial suspensions from overnight cultures of E. faecalis were irradiated during 30 seconds with the laser-lights at 1 W and 2 W of power, leaving one untreated sample as control. Surface alterations on treated E. faecalis were visualized by Atom...

  19. Control of atomic transition rates via laser light shaping

    OpenAIRE

    Jauregui, R.

    2015-01-01

    A modular systematic analysis of the feasibility of modifying atomic transition rates by tailoring the electromagnetic field of an external coherent light source is presented. The formalism considers both the center of mass and internal degrees of freedom of the atom, and all properties of the field: frequency, angular spectrum, and polarization. General features of recoil effects for internal forbidden transitions are discussed. A comparative analysis of different structured light sources is...

  20. ÉTUDE DES PROPRIÉTÉS DE PROPAGATION
    D'UN LASER À ATOMES

    OpenAIRE

    Riou, Jean-Félix

    2006-01-01

    This manuscript presents various experimental and theoretical aspects concerning a specificsystem of atom optics : the atom laser. In our experiment, this one results from aBose-Einstein condensate of rubidium 87 and we thus initially detail the various coolingtechniques used to obtain this coherent atomic source in a hybrid ferromagnetic trap.The atom lasers we produce are extracted from the condensed cloud by radiofrequency,and propagate vertically under the effect of gravity. One specifici...